Sample records for absorbing aerosols dust

  1. Modeling the Absorbing Aerosol Index

    NASA Technical Reports Server (NTRS)

    Penner, Joyce; Zhang, Sophia

    2003-01-01

    We propose a scheme to model the absorbing aerosol index and improve the biomass carbon inventories by optimizing the difference between TOMS aerosol index (AI) and modeled AI with an inverse model. Two absorbing aerosol types are considered, including biomass carbon and mineral dust. A priori biomass carbon source was generated by Liousse et al [1996]. Mineral dust emission is parameterized according to surface wind and soil moisture using the method developed by Ginoux [2000]. In this initial study, the coupled CCM1 and GRANTOUR model was used to determine the aerosol spatial and temporal distribution. With modeled aerosol concentrations and optical properties, we calculate the radiance at the top of the atmosphere at 340 nm and 380 nm with a radiative transfer model. The contrast of radiance at these two wavelengths will be used to calculate AI. Then we compare the modeled AI with TOMS AI. This paper reports our initial modeling for AI and its comparison with TOMS Nimbus 7 AI. For our follow-on project we will model the global AI with aerosol spatial and temporal distribution recomputed from the IMPACT model and DAO GEOS-1 meteorology fields. Then we will build an inverse model, which applies a Bayesian inverse technique to optimize the agreement of between model and observational data. The inverse model will tune the biomass burning source strength to reduce the difference between modelled AI and TOMS AI. Further simulations with a posteriori biomass carbon sources from the inverse model will be carried out. Results will be compared to available observations such as surface concentration and aerosol optical depth.

  2. The optical properties of absorbing aerosols with fractal soot aggregates: Implications for aerosol remote sensing

    NASA Astrophysics Data System (ADS)

    Cheng, Tianhai; Gu, Xingfa; Wu, Yu; Chen, Hao; Yu, Tao

    2013-08-01

    Applying sphere aerosol models to replace the absorbing fine-sized dominated aerosols can potentially result in significant errors in the climate models and aerosol remote sensing retrieval. In this paper, the optical properties of absorbing fine-sized dominated aerosol were modeled, which are taking into account the fresh emitted soot particles (agglomerates of primary spherules), aged soot particles (semi-externally mixed with other weakly absorbing aerosols), and coarse aerosol particles (dust particles). The optical properties of the individual fresh and aged soot aggregates are calculated using the superposition T-matrix method. In order to quantify the morphology effect of absorbing aerosol models on the aerosol remote sensing retrieval, the ensemble averaged optical properties of absorbing fine-sized dominated aerosols are calculated based on the size distribution of fine aerosols (fresh and aged soot) and coarse aerosols. The corresponding optical properties of sphere absorbing aerosol models using Lorenz-Mie solutions were presented for comparison. The comparison study demonstrates that the sphere absorbing aerosol models underestimate the absorption ability of the fine-sized dominated aerosol particles. The morphology effect of absorbing fine-sized dominated aerosols on the TOA radiances and polarized radiances is also investigated. It is found that the sphere aerosol models overestimate the TOA reflectance and polarized reflectance by approximately a factor of 3 at wavelength of 0.865 μm. In other words, the fine-sized dominated aerosol models can cause large errors in the retrieved aerosol properties if satellite reflectance measurements are analyzed using the conventional Mie theory for spherical particles.

  3. Modelling absorbing aerosol with ECHAM-HAM: Insights from regional studies

    NASA Astrophysics Data System (ADS)

    Tegen, Ina; Heinold, Bernd; Schepanski, Kerstin; Banks, Jamie; Kubin, Anne; Schacht, Jacob

    2017-04-01

    Quantifying distributions and properties of absorbing aerosol is a basis for investigations of interactions of aerosol particles with radiation and climate. While evaluations of aerosol models by field measurements can be particularly successful at the regional scale, such results need to be put into a global context for climate studies. We present an overview over studies performed at the Leibniz Institute for Tropospheric Research aiming at constraining the properties of mineral dust and soot aerosol in the global aerosol model ECHAM6-HAM2 based on different regional studies. An example is the impact of different sources for dust transported to central Asia, which is influenced, by far-range transport of dust from Arabia and the Sahara together with dust from local sources. Dust types from these different source regions were investigated in the context of the CADEX project and are expected to have different optical properties. For Saharan dust, satellite retrievals from MSG SEVIRI are used to constrain Saharan dust sources and optical properties. In the Arctic region, on one hand dust aerosol is simulated in the framework of the PalMod project. On the other hand aerosol measurements that will be taken during the DFG-funded (AC)3 field campaigns will be used to evaluate the simulated transport pathways of soot aerosol from European, North American and Asian sources, as well as the parameterization of soot ageing processes in ECHAM6-HAM2. Ultimately, results from these studies will improve the representation of aerosol absorption in the global model.

  4. Absorbing Aerosols Workshop, January 20-21, 2016

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nasiri, Shaima; Williamson, Ashley; Cappa, Christopher D.

    2016-07-01

    A workshop was held at DOE Headquarters on January 20-21, 2016 during which experts within and outside DOE were brought together to identify knowledge gaps in modeling and measurement of the contribution of absorbing aerosols (AA) to radiative forcing. Absorbing aerosols refer to those aerosols that absorb light, whereby they both reduce the amount of sunlight reaching the surface (direct effect) and heat their surroundings. By doing so, they modify the vertical distribution of heat in the atmosphere and affect atmospheric thermodynamics and stability, possibly hastening cloud drop evaporation, and thereby affecting cloud amount, formation, dissipation and, ultimately, precipitation. Depositionmore » of AA on snow and ice reduces surface albedo leading to accelerated melt. The most abundant AA type is black carbon (BC), which results from combustion of fossil fuel and biofuel. The other key AA types are brown carbon (BrC), which also results from combustion of fossil fuel and biofuel, and dust (crustal material). Each of these sources may result from, and be strongly influenced by, anthropogenic activities. The properties and amounts of AA depend upon various factors, primarily fuel source and burn conditions (e.g., internal combustion engine, flaming or smoldering wildfire), vegetation type (in the case of BC and BrC), and in the case of dust, soil type and ground cover (i.e., vegetation, snow, etc.). After emission, AA undergo chemical processing in the atmosphere that affects their physical and chemical properties. Thus, attribution of sources of AA, and understanding processes AA undergo during their atmospheric lifetimes, are necessary to understand how they will behave in a changing climate.« less

  5. A Long-term Record of Saharan Dust Aerosol Properties from TOMS Observations: Optical Depth and Single Scattering Albedo

    NASA Technical Reports Server (NTRS)

    Torres, Omar; Bhartia, P. K.; Herman, J. R.; Einaudi, Franco (Technical Monitor)

    2000-01-01

    The interaction between the strong Rayleigh scattering in the near UV spectral region (330-380 nm) and the processes of aerosol absorption and scattering, produce a clear spectral signal in the upwelling radiance at the top of the atmosphere. This interaction is the basis of the TOMS (Total Ozone Mapping Spectrometer) aerosol retrieval technique that can be used for their characterization and to differentiate non-absorbing sulfates from strongly UV-absorbing aerosols such as mineral dust. For absorbing aerosols, the characterization is in terms of the optical depth and single scattering albedo with assumptions about the aerosol plume height. The results for non-absorbing aerosols are not dependent on plume height. Although iron compounds represent only between 5% to 8% of desert dust aerosol mass, hematite (Fe2O3) accounts for most of the near UV absorption. Because of the large ultraviolet absorption characteristic of hematite, the near UV method of aerosol sensing is especially suited for the detection and characterization of desert dust aerosols. Using the combined record of near UV measurements by the Nimbus7 (1978-1992) and Earth Probe (1996-present) TOMS instruments, a global longterm climatology of near UV optical depth and single scattering albedo has been produced. The multi-year long record of mineral aerosol properties over the area of influence of the Saharan desert, will be discussed.

  6. Development of absorbing aerosol index simulator based on TM5-M7

    NASA Astrophysics Data System (ADS)

    Sun, Jiyunting; van Velthoven, Peter; Veefkind, Pepijn

    2017-04-01

    Aerosols alter the Earth's radiation budget directly by scattering and absorbing solar and thermal radiation, or indirectly by perturbing clouds formation and lifetime. These mechanisms offset the positive radiative forcing ascribed to greenhouse gases. In particular, absorbing aerosols such as black carbon and dust strongly enhance global warming. To quantify the impact of absorbing aerosol on global radiative forcing is challenging. In spite of wide spatial and temporal coverage space-borne instruments (we will use the Ozone Monitoring Instrument, OMI) are unable to derive complete information on aerosol distribution, composition, etc. The retrieval of aerosol optical properties also partly depends on additional information derived from other measurements or global atmospheric chemistry models. Common quantities of great interest presenting the amount of absorbing aerosol are AAOD (absorbing aerosol optical depth), the extinction due to absorption of aerosols under cloud free conditions; and AAI (absorbing aerosol index), a measure of aerosol absorption more directly derivable from UV band observations than AAOD. When comparing model simulations and satellite observations, resemblance is good in terms of the spatial distribution of both parameters. However, the quantitative discrepancy is considerable, indicating possible underestimates of simulated AAI by a factor of 2 to 3. Our research, hence, has started by evaluating to what extent aerosol models, such as our TM5-M7 model, represent the satellite measurements and by identifying the reasons for discrepancies. As a next step a transparent methodology for the comparison between model simulations and satellite observations is under development in the form of an AAI simulator based on TM5-M7.

  7. Summer Dust Aerosols Detected from CALIPSO Observations over the Tibetan Plateau

    NASA Technical Reports Server (NTRS)

    Huang, Jianping; Minnis, Patrick; Yi, Yuhong; Tang, Qiang; Wang, Xin; Hu, Yongxiang; Liu, Zhaoyan; Ayers, Kirk; Trepte, Charles; Winker, David

    2007-01-01

    Summertime Tibetan dust aerosol plumes are detected from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite. CALIPSO reveals that dust storms occur 4 times more frequently than previously found from Tibetan surface observations because few surface sites were available over remote northwestern Tibet. The Tibetan dust aerosol is characterized by column-averaged depolarization and color ratios around 21% and 0.83, respectively. The dust layers appear most frequently around 4-7 km above mean sea level. The depolarization ratio for about 90% of the dust particles is less than 10% at low altitudes (3-5 km), while only about 50% of the particles have a greater depolarization ratio at higher altitudes (7-10 km) suggesting a separation of larger irregular particles from smaller, near spherical ones during transport. The 4-day back trajectory analyses show that these plumes probably originate from the nearby Taklimakan desert surface and accumulate over the northern slopes of the Tibetan Plateau. These dust outbreaks can affect the radiation balance of the atmosphere of Tibet because they both absorb and reflect solar radiation.

  8. Aerosol Absorption by Black Carbon and Dust: Implications of Climate Change and Air Quality in Asia

    NASA Technical Reports Server (NTRS)

    Chin, Mian

    2010-01-01

    Atmospheric aerosol distributions from 2000 to 2007 are simulated with the global model GOCART to attribute light absorption by aerosol to its composition and sources. We show the seasonal and interannual variations of absorbing aerosols in the atmosphere over Asia, mainly black carbon and dust. and their linkage to the changes of anthropogenic and dust emissions in the region. We compare our results with observations from satellite and ground-based networks, and estimate the importance of black carbon and dust on regional climate forcing and air quality.

  9. Extending 'Deep Blue' aerosol retrieval coverage to cases of absorbing aerosols above clouds: sensitivity analysis and first case studies

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Sayer, Andrew M.; Hsu, C.; Bettenhausen, Corey

    Cases of absorbing aerosols above clouds (AAC), such as smoke or mineral dust, are omitted from most routinely-processed space-based aerosol optical depth (AOD) data products, including those from the Moderate Resolution Imaging Spectroradiometer (MODIS). This study presents a sensitivity analysis and preliminary algorithm to retrieve above-cloud AOD and liquid cloud optical depth (COD) for AAC cases from MODIS or similar

  10. Extending "Deep Blue" Aerosol Retrieval Coverage to Cases of Absorbing Aerosols Above Clouds: Sensitivity Analysis and First Case Studies

    NASA Technical Reports Server (NTRS)

    Sayer, A. M.; Hsu, N. C.; Bettenhausen, C.; Lee, J.; Redemann, J.; Schmid, B.; Shinozuka, Y.

    2016-01-01

    Cases of absorbing aerosols above clouds (AACs), such as smoke or mineral dust, are omitted from most routinely processed space-based aerosol optical depth (AOD) data products, including those from the Moderate Resolution Imaging Spectroradiometer (MODIS). This study presents a sensitivity analysis and preliminary algorithm to retrieve above-cloud AOD and liquid cloud optical depth (COD) for AAC cases from MODIS or similar sensors, for incorporation into a future version of the "Deep Blue" AOD data product. Detailed retrieval simulations suggest that these sensors should be able to determine AAC AOD with a typical level of uncertainty approximately 25-50 percent (with lower uncertainties for more strongly absorbing aerosol types) and COD with an uncertainty approximately10-20 percent, if an appropriate aerosol optical model is known beforehand. Errors are larger, particularly if the aerosols are only weakly absorbing, if the aerosol optical properties are not known, and the appropriate model to use must also be retrieved. Actual retrieval errors are also compared to uncertainty envelopes obtained through the optimal estimation (OE) technique; OE-based uncertainties are found to be generally reasonable for COD but larger than actual retrieval errors for AOD, due in part to difficulties in quantifying the degree of spectral correlation of forward model error. The algorithm is also applied to two MODIS scenes (one smoke and one dust) for which near-coincident NASA Ames Airborne Tracking Sun photometer (AATS) data were available to use as a ground truth AOD data source, and found to be in good agreement, demonstrating the validity of the technique with real observations.

  11. Extending "Deep Blue" aerosol retrieval coverage to cases of absorbing aerosols above clouds: Sensitivity analysis and first case studies

    NASA Astrophysics Data System (ADS)

    Sayer, A. M.; Hsu, N. C.; Bettenhausen, C.; Lee, J.; Redemann, J.; Schmid, B.; Shinozuka, Y.

    2016-05-01

    Cases of absorbing aerosols above clouds (AACs), such as smoke or mineral dust, are omitted from most routinely processed space-based aerosol optical depth (AOD) data products, including those from the Moderate Resolution Imaging Spectroradiometer (MODIS). This study presents a sensitivity analysis and preliminary algorithm to retrieve above-cloud AOD and liquid cloud optical depth (COD) for AAC cases from MODIS or similar sensors, for incorporation into a future version of the "Deep Blue" AOD data product. Detailed retrieval simulations suggest that these sensors should be able to determine AAC AOD with a typical level of uncertainty ˜25-50% (with lower uncertainties for more strongly absorbing aerosol types) and COD with an uncertainty ˜10-20%, if an appropriate aerosol optical model is known beforehand. Errors are larger, particularly if the aerosols are only weakly absorbing, if the aerosol optical properties are not known, and the appropriate model to use must also be retrieved. Actual retrieval errors are also compared to uncertainty envelopes obtained through the optimal estimation (OE) technique; OE-based uncertainties are found to be generally reasonable for COD but larger than actual retrieval errors for AOD, due in part to difficulties in quantifying the degree of spectral correlation of forward model error. The algorithm is also applied to two MODIS scenes (one smoke and one dust) for which near-coincident NASA Ames Airborne Tracking Sun photometer (AATS) data were available to use as a ground truth AOD data source, and found to be in good agreement, demonstrating the validity of the technique with real observations.

  12. Amplification of ENSO Effects on Indian Summer Monsoon by Absorbing Aerosols

    NASA Technical Reports Server (NTRS)

    Kim, Maeng-Ki; Lau, William K. M.; Kim, Kyu-Myong; Sang, Jeong; Kim, Yeon-Hee; Lee, Woo-Seop

    2015-01-01

    In this study, we present observational evidence, based on satellite aerosol measurements and MERRA reanalysis data for the period 1979-2011, indicating that absorbing aerosols can have strong influence on seasonal-to-interannual variability of the Indian summer monsoon rainfall, including amplification of ENSO effects. We find a significant correlation between ENSO (El Nino Southern Oscillation) and aerosol loading in April-May, with La Nina (El Nino) conditions favoring increased (decreased) aerosol accumulation over northern India, with maximum aerosol optical depth (AOD) over the Arabian Sea and Northwestern India, indicative of strong concentration of dust aerosols transported from West Asia and Middle East deserts. Composite analyses based on a normalized aerosol index (NAI) show that high concentration of aerosol over northern India in April-May is associated with increased moisture transport, enhanced dynamically induced warming of the upper troposphere over the Tibetan Plateau, and enhanced rainfall over northern India and the Himalayan foothills during May-June, followed by a subsequent suppressed monsoon rainfall over all India,consistent with the Elevated Heat Pump (EHP) hypothesis (Lau et al. 2006). Further analyses from sub-sampling of ENSO years, with normal (less than 1 sigma), and abnormal (greater than 1 sigma)) NAI over northern India respectively show that the EHP may lead to an amplification of the Indian summer monsoon response to ENSO forcing, particularly with respect to the increased rainfall over the Himalayan foothills, and the warming of the upper troposphere over the Tibetan Plateau. Our results suggest that absorbing aerosol, particular desert dusts can strongly modulate ENSO influence, and possibly play important roles as a feedback agent in climate change in Asian monsoon regions.

  13. Assessment of capabilities of multiangle imaging photo-polarimetry for atmospheric correction in presence of absorbing aerosols

    NASA Astrophysics Data System (ADS)

    Kalashnikova, O. V.; Garay, M. J.; Xu, F.; Seidel, F. C.; Diner, D. J.

    2015-12-01

    Satellite remote sensing of ocean color is a critical tool for assessing the productivity of marine ecosystems and monitoring changes resulting from climatic or environmental influences. Yet water-leaving radiance comprises less than 10% of the signal measured from space, making correction for absorption and scattering by the intervening atmosphere imperative. Traditional ocean color retrieval algorithms utilize a standard set of aerosol models and the assumption of negligible water-leaving radiance in the near-infrared. Modern improvements have been developed to handle absorbing aerosols such as urban particulates in coastal areas and transported desert dust over the open ocean, where ocean fertilization can impact biological productivity at the base of the marine food chain. Even so, imperfect knowledge of the absorbing aerosol optical properties or their height distribution results in well-documented sources of error. In the UV, the problem of UV-enhanced absorption and nonsphericity of certain aerosol types are amplified due to the increased Rayleigh and aerosol optical depth, especially at off-nadir view angles. Multi-angle spectro-polarimetric measurements have been advocated as an additional tool to better understand and retrieve the aerosol properties needed for atmospheric correction for ocean color retrievals. The central concern of the work to be described is the assessment of the effects of absorbing aerosol properties on water leaving radiance measurement uncertainty by neglecting UV-enhanced absorption of carbonaceous particles and by not accounting for dust nonsphericity. In addition, we evaluate the polarimetric sensitivity of absorbing aerosol properties in light of measurement uncertainties achievable for the next generation of multi-angle polarimetric imaging instruments, and demonstrate advantages and disadvantages of wavelength selection in the UV/VNIR range. The phase matrices for the spherical smoke particles were calculated using a standard

  14. Impact of Radiatively Interactive Dust Aerosols in the NASA GEOS-5 Climate Model: Sensitivity to Dust Particle Shape and Refractive Index

    NASA Technical Reports Server (NTRS)

    Colarco, Peter R.; Nowottnick, Edward Paul; Randles, Cynthia A.; Yi, Bingqi; Yang, Ping; Kim, Kyu-Myong; Smith, Jamison A.; Bardeen, Charles D.

    2013-01-01

    We investigate the radiative effects of dust aerosols in the NASA GEOS-5 atmospheric general circulation model. GEOS-5 is improved with the inclusion of a sectional aerosol and cloud microphysics module, the Community Aerosol and Radiation Model for Atmospheres (CARMA). Into CARMA we introduce treatment of the dust and sea salt aerosol lifecycle, including sources, transport evolution, and sinks. The aerosols are radiatively coupled to GEOS-5, and we perform a series of multi-decade AMIP-style simulations in which dust optical properties (spectral refractive index and particle shape distribution) are varied. Optical properties assuming spherical dust particles are from Mie theory, while those for non-spherical shape distributions are drawn from a recently available database for tri-axial ellipsoids. The climatologies of the various simulations generally compare well to data from the MODIS, MISR, and CALIOP space-based sensors, the ground-based AERONET, and surface measurements of dust deposition and concentration. Focusing on the summertime Saharan dust cycle we show significant variability in our simulations resulting from different choices of dust optical properties. Atmospheric heating due to dust enhances surface winds over important Saharan dust sources, and we find a positive feedback where increased dust absorption leads to increased dust emissions. We further find that increased dust absorption leads to a strengthening of the summertime Hadley cell circulation, increasing dust lofting to higher altitudes and strengthening the African Easterly Jet. This leads to a longer atmospheric residence time, higher altitude, and generally more northward transport of dust in simulations with the most absorbing dust optical properties. We find that particle shape, although important for radiance simulations, is a minor effect compared to choices of refractive index, although total atmospheric forcing is enhanced by greater than 10 percent for simulations incorporating a

  15. Modern dust aerosol availability in northwestern China.

    PubMed

    Wang, Xunming; Cheng, Hong; Che, Huizheng; Sun, Jimin; Lu, Huayu; Qiang, Mingrui; Hua, Ting; Zhu, Bingqi; Li, Hui; Ma, Wenyong; Lang, Lili; Jiao, Linlin; Li, Danfeng

    2017-08-18

    The sources of modern dust aerosols and their emission magnitudes are fundamental for linking dust with climate and environment. Using field sample data, wind tunnel experiments and statistical analysis, we determined the contributions of wadis, gobi (stony desert), lakebeds, riverbeds, and interdunes to modern dust aerosol availability in the three important potential dust sources including the Tarim Basin, Qaidam Basin, and Ala Shan Plateau of China. The results show that riverbeds are the dominant landscape for modern dust aerosol availabilities in the Qaidam Basin, while wadis, gobi, and interdunes are the main landscapes over the Ala Shan Plateau and Tarim Basin. The Ala Shan Plateau and Tarim Basin are potential dust sources in northwestern China, while the Qaidam Basin is not a major source of the modern dust aerosols nowadays, and it is not acting in a significant way to the Loess Plateau presently. Moreover, most of modern dust aerosol emissions from China originated from aeolian processes with low intensities rather than from major dust events.

  16. Spatio-temporal distribution of absorbing and non-absorbing aerosols derived from Aura-OMI Aerosol Index over Greece

    NASA Astrophysics Data System (ADS)

    Kaskaoutis, D. G.; Nastos, P. T.; Kosmopoulos, P. G.; Kambezidis, H. D.; Kharol, S. K.; Badarinath, K. V. S.

    2009-04-01

    The Aerosol Index (AI) observations derived from the Ozone Monitoring Instrument (OMI) on board the Dutch-Finnish Aura satellite are analyzed over Greece covering the whole period of the OMI available data, from September 2004 to August 2008. The objective of this study was to analyze the spatial, seasonal and inter-annual variability of AI over Greece, detected by OMI during 2004-2008, with an evaluation of potential contributing factors, including precipitation and long-range transport (Sahara dust and European pollution). The AI data cover the whole Greek territory (34o-42oN, 20o-28oE) with a spatial resolution of 0.25o x 0.25o (13 km x 24 km at nadir). The results show significant spatial and temporal variability of the seasonal and monthly mean AI, with higher values at the southern parts and lower values over northern Greece. On the other hand, the AI values do not show significant differences between the western and eastern parts and, therefore, the longitude-averaged AI values can be utilized to reveal the strong south-to-north gradient. This gradient significantly changes from season to season being more intense in spring and summer, while it is minimized in winter. Another significant remark is the dominance of negative AI values over northern Greece in the summer months, indicating the presence of non-UV absorbing aerosols, such as sulfate and sea-salt particles. The great geographical extent of the negative AI values in the summer months is indicative of long-range transport of such aerosols. In contrast, the high positive AI values over south Greece, mainly in spring, clearly reveal the UV-absorbing nature of desert-dust particles affecting the area during Saharan dust events. Synoptically, the spatial distribution in OMI-AI values was related to the Saharan dust events mainly over southern Greece and to the trans-boundary-pollution transport, consisting mainly of sulfate particles, in northern Greece. The annual variation of spatial-averaged AI values

  17. Theoretical Characterization of the Radiative Properties of Dust Aerosol for the Air Force Combat Climatology Center Point Analysis Intelligence System

    DTIC Science & Technology

    2007-03-01

    dust aerosol is known to absorb radiation in these wavelengths. Therefore, the absorptive properties of the aerosol must be taken into account to...of the dust aerosol on radiation propagation is complicated. The study addressed this problem by modeling various radiative transfer situations...are ubiquitous in nature and frequently are the determining factor in the amount of radiation received at a sensor.” The horizontal and vertical

  18. Ice nucleation by soil dust compared to desert dust aerosols

    NASA Astrophysics Data System (ADS)

    Moehler, O.; Steinke, I.; Ullrich, R.; Höhler, K.; Schiebel, T.; Hoose, C.; Funk, R.

    2015-12-01

    A minor fraction of atmospheric aerosol particles, so-called ice-nucleating particles (INPs), initiates the formation of the ice phase in tropospheric clouds and thereby markedly influences the Earth's weather and climate systems. Whether an aerosol particle acts as an INP depends on its size, morphology and chemical compositions. The INP fraction of certain aerosol types also strongly depends on the temperature and the relative humidity. Because both desert dust and soil dust aerosols typically comprise a variety of different particles, it is difficult to assess and predict their contribution to the atmospheric INP abundance. This requires both accurate modelling of the sources and atmospheric distribution of atmospheric dust components and detailed investigations of their ice nucleation activities. The latter can be achieved in laboratory experiments and parameterized for use in weather and climate models as a function of temperature and particle surface area, a parameter called ice-nucleation active site (INAS) density. Concerning ice nucleation activity studies, the soil dust is of particular interest because it contains a significant fraction of organics and biological components, both with the potential for contributing to the atmospheric INP abundance at relatively high temperatures compared to mineral components. First laboratory ice nucleation experiments with a few soil dust samples indicated their INP fraction to be comparable or slightly enhanced to that of desert dust. We have used the AIDA (Aerosol Interaction and Dynamics in the Atmosphere) cloud simulation chamber to study the immersion freezing ability of four different arable soil dusts, sampled in Germany, China and Argentina. For temperatures higher than about -20°C, we found the INP fraction of aerosols generated from these samples by a dry dispersion technique to be significantly higher compared to various desert dust aerosols also investigated in AIDA experiments. In this contribution, we

  19. Using Aerosol Reflectance for Dust Detection

    NASA Astrophysics Data System (ADS)

    Bahramvash Shams, S.; Mohammadzade, A.

    2013-09-01

    In this study we propose an approach for dust detection by aerosol reflectance over arid and urban region in clear sky condition. In urban and arid areas surface reflectance in red and infrared spectral is bright and hence shorter wavelength is required for this detections. Main step of our approach can be mentioned as: cloud mask for excluding cloudy pixels from our calculation, calculate Rayleigh path radiance, construct a surface reflectance data base, estimate aerosol reflectance, detect dust aerosol, dust detection and evaluations of dust detection. Spectral with wavelength 0.66, 0.55, 0.47 μm has been used in our dust detection. Estimating surface reflectance is the most challenging step of obtaining aerosol reflectance from top of atmosphere (TOA) reflectance. Hence for surface estimation we had created a surface reflectance database of 0.05 degree latitude by 0.05 degree longitude resolution by using minimum reflectivity technique (MRT). In order to evaluate our dust detection algorithm MODIS aerosol product MOD04 and common dust detection method named Brightness Temperature Difference (BTD) had been used. We had implemented this method to Moderate Resolution Imaging Spectroradiometer (MODIS) image of part of Iran (7 degree latitude and 8 degree longitude) spring 2005 dust phenomenon from April to June. This study uses MODIS LIB calibrated reflectance high spatial resolution (500 m) MOD02Hkm on TERRA spacecraft. Hence our dust detection spatial resolution will be higher spatial resolution than MODIS aerosol product MOD04 which has 10 × 10 km2 and BTD resolution is 1 km due to the band 29 (8.7 μm), 31 (11 μm), and 32 (12 μm) spatial resolutions.

  20. MODIS Retrieval of Dust Aerosol

    NASA Technical Reports Server (NTRS)

    Remer, Lorraine A.; Kaufman, Yoram J.; Tanre, Didier

    2003-01-01

    The MODerate resolution Imaging Spectroradiometer (MODIS) currently aboard both the Terra and Aqua satellites produces a suite of products designed to characterize global aerosol distribution, optical thickness and particle size. Never before has a space-borne instrument been able to provide such detailed information, operationally, on a nearly global basis every day. The three years of Terra-MODIS data have been validated by comparing with co-located AERONET observations of aerosol optical thickness and derivations of aerosol size parameters. Some 8000 comparison points located at 133 AERONET sites around the globe show that the MODIS aerosol optical thickness retrievals are accurate to within the pre-launch expectations. However, the validation in regions dominated by desert dust is less accurate than in regions dominated by fine mode aerosol or background marine sea salt. The discrepancy is most apparent in retrievals of aerosol size parameters over ocean. In dust situations, the MODIS algorithm tends to under predict particle size because the reflectances at top of atmosphere measured by MODIS exhibit the stronger spectral signature expected by smaller particles. This pattern is consistent with the angular and spectral signature of non-spherical particles. All possible aerosol models in the MODIS Look-Up Tables were constructed from Mie theory, assuming a spherical shape. Using a combination of MODIS and AERONET observations, in regimes dominated by desert dust, we construct phase functions, empirically, with no assumption of particle shape. These new phase functions are introduced into the MODIS algorithm, in lieu of the original options for large dust-like particles. The results will be analyzed and examined.

  1. Absorbing Aerosols Above Cloud: Detection, Quantitative Retrieval, and Radiative Forcing from Satellite-based Passive Sensors

    NASA Astrophysics Data System (ADS)

    Jethva, H.; Torres, O.; Remer, L. A.; Bhartia, P. K.

    2012-12-01

    Light absorbing particles such as carbonaceous aerosols generated from biomass burning activities and windblown dust particles can exert a net warming effect on climate; the strength of which depends on the absorption capacity of the particles and brightness of the underlying reflecting background. When advected over low-level bright clouds, these aerosols absorb the cloud reflected radiation from ultra-violet (UV) to shortwave-IR (SWIR) and makes cloud scene darker-a phenomenon commonly known as "cloud darkening". The apparent "darkening" effect can be seen by eyes in satellite images as well as quantitatively in the spectral reflectance measurements made by space borne sensors over regions where light absorbing carbonaceous and dust aerosols overlay low-level cloud decks. Theoretical radiative transfer simulations support the observational evidence, and further reveal that the strength of the cloud darkening and its spectral signature (or color ratio) between measurements at two wavelengths are a bi-function of aerosol and cloud optical thickness (AOT and COT); both are measures of the total amount of light extinction caused by aerosols and cloud, respectively. Here, we developed a retrieval technique, named as the "color ratio method" that uses the satellite measurements at two channels, one at shorter wavelength in the visible and one at longer wavelength in the shortwave-IR for the simultaneous retrieval of AOT and COT. The present technique requires assumptions on the aerosol single-scattering albedo and aerosol-cloud separation which are supplemented by the Aerosol Robotic Network (AERONET) and space borne CALIOP lidar measurements. The retrieval technique has been tested making use of the near-UV and visible reflectance observations made by the Ozone Monitoring Instrument (OMI) and Moderate Resolution Imaging Spectroradiometer (MODIS) for distinct above-cloud smoke and dust aerosol events observed seasonally over the southeast and tropical Atlantic Ocean

  2. Effects of Absorbing Aerosols on Accelerated Melting of Snowpack in the Tibetan-Himalayas Region

    NASA Technical Reports Server (NTRS)

    Lau, William K. M.

    2011-01-01

    The impacts of absorbing aerosol on melting of snowpack in the Hindu-Kush-Tibetan-Himalayas (HKTH) region are studied using NASA satellite and GEOS-5 GCM. Results from GCM experiments shows that a 8-10% in the rate of melting of snowpack over the western Himalayas and Tibetan Plateau can be attributed to the aerosol elevated-heat-pump (EHP) feedback effect (Lau et al. 2008), initiated by the absorption of solar radiation by absorbing aerosols accumulated over the Indo-Gangetic Plain and Himalayas foothills. On the other hand, deposition of black carbon on snow surface was estimated to give rise to a reduction in snow surface albedo of 2 - 5%, and an increased annual runoff of 9-24%. From case studies using satellite observations and re-analysis data, we find consistent signals of possible impacts of dust and black carbon aerosol in blackening snow surface, in accelerating spring melting of snowpack in the HKHT, and consequentially in influencing shifts in long-term Asian summer monsoon rainfall pattern.

  3. A Ten-Year Global Record of Absorbing Aerosols Above Clouds from OMI's Near-UV Observations

    NASA Technical Reports Server (NTRS)

    Jethva, Hiren; Torres, Omar; Ahn, Changwoo

    2016-01-01

    Aerosol-cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of an adequate knowledge of the complex microphysical and radiative processes associated with the aerosol-cloud system. The situations when aerosols and clouds are found in the same atmospheric column, for instance, when light-absorbing aerosols such as biomass burning generated carbonaceous particles or wind-blown dust overlay low-level cloud decks, are commonly found over several regional of the world. Contrary to the cloud-free scenario over dark surface, for which aerosols are known to produce a net cooling effect (negative radiative forcing) on climate, the overlapping situation of absorbing aerosols over cloud can potentially exert a significant level of atmospheric absorption and produces a positive radiative forcing at top-of-atmosphere. The magnitude of direct radiative effects of aerosols above cloud depends directly on the aerosol loading, microphysical-optical properties of the aerosol layer and the underlying cloud deck, and geometric cloud fraction. We help in addressing this problem by introducing a novel product of optical depth of absorbing aerosols above clouds retrieved from near-UV observations made by the Ozone Monitoring Instrument (OMI) on board NASA's Aura platform. The presence of absorbing aerosols above cloud reduces the upwelling radiation reflected by cloud and produces a strong 'color ratio' effect in the near-UV region, which can be unambiguously detected in the OMI measurements. Physically based on this effect, the OMACA algorithm retrieves the optical depths of aerosols and clouds simultaneously under a prescribed state of atmosphere. The algorithm architecture and results from a ten-year global record including global climatology of frequency of occurrence and above-cloud aerosol optical depth, and a discussion on related future field campaigns are presented.

  4. Is It Possible to Distinguish Between Dust and Salt Aerosol Over Waters with Unknown Chlorophyll Concentrations Using Spectral Remote Sensing?

    NASA Technical Reports Server (NTRS)

    Levy, R. C.; Kaufman, Y. J.

    1999-01-01

    Atmospheric aerosol has uncertain impacts on the global climate system, as well as on atmospheric and bio-geo-chemical processes of regional and local scales. EOS-MODIS is one example of a satellite sensor designed to improve understanding of the aerosols' type, size and distribution at all temporal and spatial scales. Ocean scientists also plan to use data from EOS-MODIS to assess the temporal and spatial coverage of in-water chlorophyll. MODIS is the first sensor planned to observe the combined ocean-atmosphere system with a wide spectral range (from 410 to 2200 nm). Dust aerosol and salt aerosol have similar spectral signals for wavelengths longer than 550 nm, but because dust selectively absorbs blue light, they have divergent signals in the blue wavelength regions (412 to 490 nm). Chlorophyll also selectively absorbs blue radiation, so that varying chlorophyll concentrations produces a highly varying signal in the blue regions, but less variability in the green, and almost no signal in the red to mid-infrared regions. Thus, theoretically, it may be difficult to differentiate dust and salt in the presence of unknown chlorophyll in the ocean. This study attempts to address the cases in which aerosol and chlorophyll signals can and cannot be separated. For the aerosol spectra, we use the aerosol lookup table from the operational MODIS aerosol-over-ocean algorithm, and for chlorophyll spectra, we use the SeaBAM data set (created for SeaWiFS). We compare the signals using Principal Component Analysis and attempt to retrieve both chlorophyll and aerosol properties using a variant of the operational MODIS aerosol-over-ocean algorithm. Results show that for small optical depths, less than 0.5, it is not possible to differentiate between dust and salt and to determine the chlorophyll concentration at the same time. For larger aerosol optical depths, the chlorophyll signals are comparatively insignificant, and we can hope to distinguish between dust and salt.

  5. Role of near ultraviolet wavelength measurements in the detection and retrieval of absorbing aerosols from space

    NASA Astrophysics Data System (ADS)

    Mukai, Sonoyo; Fujito, Toshiyuki; Nakata, Makiko; Sano, Itaru

    2017-10-01

    Aerosol remote sensing by ultraviolet (UV) wavelength is established by a Total Ozone Mapping Spectrometer (TOMS) mounted on the long-life satellite Nimbus-7 and continues to make observations using Ozone monitoring instrument (OMI) located on the Aura satellite. For example, TOMS demonstrated that UV radiation (0.331 and 0.360 μm) could easily detect absorbing particles such as mineral dust or smoke aerosols. TOMS-AI (absorbing aerosol index) has been used to identify the absorbing aerosols from space. For an upcoming mission, JAXA/GCOM-C will have the polarization sensor SGLI boarded in December 2017. The SGLI has multi (19)-channels including near UV (0.380 μm) and violet (0.412 μm) wavelengths. This work intends to examine the role of near UV data in the detection of absorbing aerosols similar to TOMS-AI played. In practice, the measurements by GLI mounted on the short Japanese mission JAXA/ADEOS-2, whose data archive period was just 8 months from April to October in 2003, are available for simulation of SGLI data because ADEOS-2/GLI installed near UV and violet channels. First of all, the ratio of data at 0.412 μm to that at 0.380 μm is examined as an indicator to detect absorbing aerosols on a global scale during ADEOS-2 era. It is noted that our research group has developed an efficient algorithm for aerosol retrieval in hazy episodes (dense concentrations of atmospheric aerosols). It can be said that at least this work is an attempt to grasp the biomass burning plumes from the satellite.

  6. A Global, Decadal, Quantitative Record of Absorbing Aerosols above Cloud Using OMI's Near-UV Observations

    NASA Astrophysics Data System (ADS)

    Torres, O.; Jethva, H. T.; Ahn, C.

    2016-12-01

    Aerosol-cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of an adequate knowledge of the complex microphysical and radiative processes of the aerosol-cloud system. The situations when aerosols and clouds are found in the same atmospheric column, for instance, when light-absorbing aerosols such as biomass burning generated carbonaceous particles or wind-blown dust overlay low-level cloud decks, are commonly found over several regions of the world. Contrary to the known cooling effects of these aerosols in cloud-free scenario over dark surface, the overlapping situation of absorbing aerosols over cloud can potentially exert a significant level of atmospheric absorption and produces a positive radiative forcing (warming) at top-of-atmosphere. The magnitude of direct radiative effects of aerosols above cloud directly depends on the aerosol loading, microphysical and optical properties of the aerosol layer and the underlying cloud deck, and geometric cloud fraction. We help in addressing this problem by introducing a novel product of above-cloud aerosol optical depth (ACAOD) of absorbing aerosols retrieved from near-UV observations made by the Ozone Monitoring Instrument (OMI) on board NASA's Aura platform. Physically based on the strong `color ratio' effect in the near-UV caused by the spectral absorption of aerosols above cloud, the algorithm, formally named as OMACA, retrieves the optical depths of aerosols and clouds simultaneously under a prescribed state of atmosphere. Here, we present the algorithm architecture and results from an 11-year global record (2005-2015) including global climatology of frequency of occurrence and ACAOD. The theoretical uncertainty analysis and planned validation activities using measurements from upcoming field campaigns are also discussed.

  7. Analysis of reflectance spectra of UV-absorbing aerosol scenes measured by SCIAMACHY

    NASA Astrophysics Data System (ADS)

    de Graaf, M.; Stammes, P.; Aben, E. A. A.

    2007-01-01

    Reflectance spectra from 280-1750 nm of typical desert dust aerosol (DDA) and biomass burning aerosol (BBA) scenes over oceans are presented, measured by the space-borne spectrometer Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY). DDA and BBA are both UV-absorbing aerosols, but their effect on the top-of-atmosphere (TOA) reflectance is different due to differences in the way mineral aerosols and smoke reflect and absorb radiation. Mineral aerosols are typically large, inert particles, found in warm, dry continental air. Smoke particles, on the other hand, are usually small particles, although often clustered, chemically very active and highly variable in composition. Moreover, BBA are hygroscopic and over oceans BBA were invariably found in cloudy scenes. TOA reflectance spectra of typical DDA and BBA scenes were analyzed, using radiative transfer simulations, and compared. The DDA spectrum was successfully simulated using a layer with a bimodal size distribution of mineral aerosols in a clear sky. The spectrum of the BBA scene, however, was determined by the interaction between cloud droplets and smoke particles, as is shown by simulations with a model of separate aerosol and cloud layers and models with internally and externally mixed aerosol/cloud layers. The occurrence of clouds in smoke scenes when sufficient water vapor is present usually prevents the detection of optical properties of these aerosol plumes using space-borne sensors. However, the Absorbing Aerosol Index (AAI), a UV color index, is not sensitive to scattering aerosols and clouds and can be used to detect these otherwise obscured aerosol plumes over clouds. The amount of absorption of radiation can be expressed using the absorption optical thickness. The absorption optical thickness in the DDA case was 0.42 (340 nm) and 0.14 (550 nm) for an aerosol layer of optical thickness 1.74 (550 nm). In the BBA case the absorption optical thickness was 0.18 (340 nm) and 0

  8. Sensitivity of multiangle photo-polarimetry to absorbing aerosol vertical layering and properties: Quantifying measurement uncertainties for ACE requirements

    NASA Astrophysics Data System (ADS)

    Kalashnikova, O. V.; Garay, M. J.; Davis, A. B.; Natraj, V.; Diner, D. J.; Tanelli, S.; Martonchik, J. V.; JPl Team

    2011-12-01

    The impact of tropospheric aerosols on climate can vary greatly based upon relatively small variations in aerosol properties, such as composition, shape and size distributions, as well as vertical layering. Multi-angle polarimetric measurements have been advocated in recent years as an additional tool to better understand and retrieve the aerosol properties needed for improved predictions of aerosol radiative forcing on climate. The central concern of this work is the assessment of the effects of absorbing aerosol properties under measurement uncertainties achievable for future generation multi-angle, polarimetric imaging instruments under ACE mission requirements. As guidelines, the on-orbit performance of MISR for multi-angle intensity measurements and the reported polarization sensitivities of a MSPI prototype were adopted. In particular, we will focus on sensitivities to absorbing aerosol layering and observation-constrained refractive indices (resulting in various single scattering albedos (SSA)) of both spherical and non-spherical absorbing aerosol types. We conducted modeling experiments to determine how the measured Stokes vector elements are affected in UV-NIR range by the vertical distribution, mixing and layering of smoke and dust aerosols, and aerosol SSA under the assumption of a black and polarizing ocean surfaces. We use a vector successive-orders-of-scattering (SOS) and VLIDORT transfer codes that show excellent agreement. Based on our sensitivity studies we will demonstrate advantages and disadvantages of wavelength selection in UV-NIR range to access absorbing aerosol properties. Polarized UV channels do not show particular advantage for absorbing aerosol property characterization due to dominating molecular signal. Polarimetric SSA sensitivity is small, however needed to be considered in the future polarimetric retrievals under ACE-defined uncertainty.

  9. Role of absorbing aerosols on hot extremes in India in a GCM

    NASA Astrophysics Data System (ADS)

    Mondal, A.; Sah, N.; Venkataraman, C.; Patil, N.

    2017-12-01

    Temperature extremes and heat waves in North-Central India during the summer months of March through June are known for causing significant impact in terms of human health, productivity and mortality. While greenhouse gas-induced global warming is generally believed to intensify the magnitude and frequency of such extremes, aerosols are usually associated with an overall cooling, by virtue of their dominant radiation scattering nature, in most world regions. Recently, large-scale atmospheric conditions leading to heat wave and extreme temperature conditions have been analysed for the North-Central Indian region. However, the role of absorbing aerosols, including black carbon and dust, is still not well understood, in mediating hot extremes in the region. In this study, we use 30-year simulations from a chemistry-coupled atmosphere-only General Circulation Model (GCM), ECHAM6-HAM2, forced with evolving aerosol emissions in an interactive aerosol module, along with observed sea surface temperatures, to examine large-scale and mesoscale conditions during hot extremes in India. The model is first validated with observed gridded temperature and reanalysis data, and is found to represent observed variations in temperature in the North-Central region and concurrent large-scale atmospheric conditions during high temperature extremes realistically. During these extreme events, changes in near surface properties include a reduction in single scattering albedo and enhancement in short-wave solar heating rate, compared to climatological conditions. This is accompanied by positive anomalies of black carbon and dust aerosol optical depths. We conclude that the large-scale atmospheric conditions such as the presence of anticyclones and clear skies, conducive to heat waves and high temperature extremes, are exacerbated by absorbing aerosols in North-Central India. Future air quality regulations are expected to reduce sulfate particles and their masking of GHG warming. It is

  10. African Dust Aerosols as Atmospheric Ice Nuclei

    NASA Technical Reports Server (NTRS)

    DeMott, Paul J.; Brooks, Sarah D.; Prenni, Anthony J.; Kreidenweis, Sonia M.; Sassen, Kenneth; Poellot, Michael; Rogers, David C.; Baumgardner, Darrel

    2003-01-01

    Measurements of the ice nucleating ability of aerosol particles in air masses over Florida having sources from North Africa support the potential importance of dust aerosols for indirectly affecting cloud properties and climate. The concentrations of ice nuclei within dust layers at particle sizes below 1 pn exceeded 1/cu cm; the highest ever reported with our device at temperatures warmer than homogeneous freezing conditions. These measurements add to previous direct and indirect evidence of the ice nucleation efficiency of desert dust aerosols, but also confirm their contribution to ice nuclei populations at great distances from source regions.

  11. The thermal infrared radiance properties of dust aerosol over ocean

    NASA Astrophysics Data System (ADS)

    Hao, Zengzhou; Pan, Delu; Tu, Qianguang; Gong, Fang; Chen, Jianyu

    2015-10-01

    Asian dust storms, which can long-range transport to ocean, often occur on spring. The present of Asian dust aerosols over ocean makes some difficult for other studies, such as cloud detection, and also take some advantage for ocean, such as take nutrition into the ocean by dry or wet deposition. Therefore, it is important to study the dust aerosol and retrieve the properties of dust from satellite observations that is mainly from the thermal infrared radiance. In this paper, the thermal infrared radiance properties of dust aerosol over ocean are analyzed from MODIS and MTSAT2 observations and Streamer model simulations. By analyzing some line samples and a series of dust aerosol region, it shows that the dust aerosol brightness temperature at 12μm (BT12) is always greater than BT11 and BT8.5, and BT8.5 is general greater than BT11. The brightness temperature different between 11μm and 12μm (BTD11-12) increases with the dust intensity. And the BTD11-12 will become positive when the atmospheric relative humidity is greater than 70%. The BTD11-12 increases gradually with the surface temperature while the effect on BTD11-12 of dust layer temperature is not evident. Those are caused by the transmission of the dust aerosol is different at the two thermal infrared channels. During daytime, dust infrared brightness temperature at mid-infrared bands should reduce the visual radiance, which takes about 25K or less. In general, BT3.7 is greater than BT11 for dust aerosol. Those results are helpful to monitor or retrieve dust aerosol physical properties over ocean from satellite.

  12. Contribution of dust and anthropogenic pollution to aerosol optical depth in South Korea during Spring/Summer 2016

    NASA Astrophysics Data System (ADS)

    Beyersdorf, A. J.; Corr, C.; Hite, J. R.; Jordan, C.; Nenes, A.; Thornhill, K. L., II; Winstead, E.; Anderson, B. E.

    2017-12-01

    Aerosol pollution is a major problem over the Korean peninsula during spring and summer each year. Spring coincides with peak transport of dust and biomass-burning aerosol transport from East Asia. These sources coupled with persistently high concentrations of local anthropogenic pollution and urban aerosols transported from upwind regions create complex, spatially inhomogeneous mixtures of aerosol types especially during periods of high aerosol loading. In order to improve diagnostic and forecasting capabilities for these high loading events using remote sensors and models, the NASA Korea-US Air Quality Study (KORUS-AQ) provided detailed evaluation of the vertical, spatial, and temporal variations in pollution during May and June 2016. Aerosol measurements from an instrumented aircraft are used to determine the relative abundance and properties of anthropogenic aerosol and dust in South Korea. Of particular interest are differences in the Seoul Metropolitan Area as a function of location and day. Based on preliminary analysis, aerosol over central Seoul were more absorbing than measurements east of Seoul (Taewha Forest) suggesting primary emissions dominate over Seoul while secondary aerosol production occurs as the aerosol is transported downwind. Dust transport will be determined based on a wing-mounted probe in combination with filter samples. Sub-micron anthropogenic data is more completely studied including optical and size measurements, composition, and cloud activity.

  13. Version 2.0 AERONET Dust Aerosol properties, Constraints and Application to Asian Dust Observations

    NASA Technical Reports Server (NTRS)

    Holben, Brent; Eck, Tom; Holben, Brent; Eck, Tom; Siniuk, Aliaksander; Huangand, Jianping; Zang, Wu

    2007-01-01

    In November 2006, AERONET released Version 2 of the Dubovik and King sky radiance and optical depth inversion. Reanalysis of the entire AERONET database revealed marked differences in aerosol properties in arid and semi arid regions with dust dominated aerosols. The change will be illustrated through sensitivity analysis and examples from the UAE2 (United Arab Emirates Unified Aerosol Experiment) field campaign. Properties of dust dominated aerosols will be presented from regional AERONET sites in China showing variations in dust aerosol properties. The constraints and limitations of the AERONET inversion will be presented that will facilitate analysis by the user community of these data.

  14. Understanding the impact of saharan dust aerosols on tropical cyclones

    NASA Astrophysics Data System (ADS)

    Naeger, Aaron

    Genesis of Tropical Cyclones (TCs) in the main development region for Atlantic hurricanes is tied to convection initiated by African easterly waves (AEWs) during Northern hemisphere summer and fall seasons. The main development region is also impacted by dust aerosols transported from the Sahara. It has been hypothesized that dust aerosols can modulate the development of TCs through aerosol-radiation and aerosol-cloud interaction processes. In this study, we investigate the impact of dust aerosols on TC development using the Weather Research and Forecasting model coupled with chemistry (WRF-Chem). We first develop a technique to constrain the WRF-Chem model with a realistic three-dimensional spatial distribution of dust aerosols. The horizontal distribution of dust is specified using the Moderate Resolution Imaging Spectroradiometer (MODIS) derived aerosol products and output from the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model. The vertical distribution of dust is constrained using the Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO). We validate our technique through in situ aircraft measurements where both showed aerosol number concentrations from 20-30 cm-3 in the atmosphere for Saharan dust moving over the eastern Atlantic Ocean. Then, we use the satellite data constraint technique to nudge the WRF-Chem aerosol fields throughout the simulation of TC Florence developing over the eastern Atlantic Ocean during September 2006. Three different experiments are conducted where the aerosol-radiation and aerosol-cloud interaction processes are either activated or deactivated in the model while all other model options are identical between the experiments. By comparing the model experiment results, the impact of the aerosol interaction processes on TC development can be understood. The results indicate that dust aerosols can delay or prevent the development of a TC as the minimum sea level pressure of TC Florence was 13 h

  15. Extending MODIS Deep Blue Aerosol Retrieval Coverage to Cases of Absorbing Aerosols Above Clouds: First Results

    NASA Technical Reports Server (NTRS)

    Sayer, A. M.; Hsu, N. C.; Bettenhausen, C.; Lee, J.; Redemann, J.; Shinozuka, Y.; Schmid, B.

    2015-01-01

    Absorbing smoke or mineral dust aerosols above clouds (AAC) are a frequent occurrence in certain regions and seasons. Operational aerosol retrievals from sensors like MODIS omit AAC because they are designed to work only over cloud-free scenes. However, AAC can in principle be quantified by these sensors in some situations (e.g. Jethva et al., 2013; Meyer et al., 2013). We present a summary of some analyses of the potential of MODIS-like instruments for this purpose, along with two case studies using airborne observations from the Ames Airborne Tracking Sunphotometer (AATS; http://geo.arc.nasa.gov/sgg/AATS-website/) as a validation data source for a preliminary AAC algorithm applied to MODIS measurements. AAC retrievals will eventually be added to the MODIS Deep Blue (Hsu et al., 2013) processing chain.

  16. Light-Absorbing Aerosol during NASA GRIP: Overview of Observations in the Free Troposphere and Associated with Tropical Storm Systems

    NASA Astrophysics Data System (ADS)

    Ziemba, L. D.; Beyersdorf, A. J.; Chen, G.; Corr, C. A.; Craig, L.; Dhaniyala, S.; Dibb, J. E.; Hudgins, C. H.; Ismail, S.; Latham, T.; Nenes, A.; Thornhill, K. L.; Winstead, E.; Anderson, B. E.

    2010-12-01

    Aerosols play a significant role in regulating Earth’s climate. Absorbing aerosols typically constitute a small fraction of ambient particle mass but can contribute significantly to direct and indirect climate forcing depending on size, mixing state, concentration, chemical composition, and vertical and spatial distribution. Aerosols may also significantly affect tropical storm/hurricane dynamics through direct light absorption and activation as cloud nuclei. An extensive suite of instrumentation measuring aerosol chemical, physical, and optical properties was deployed aboard the NASA DC-8 to characterize aerosol during the NASA GRIP (Genesis and Rapid Intensification Processes; August-September 2010) mission. The majority of flight time was spent at high altitude (greater than 9 km) and thus much of the sampling was done in the free troposphere, including extensive sampling in the vicinity of tropical storm systems and more diffuse cirrus clouds. With operations based in Fort Lauderdale, FL and St. Croix, U.S. Virgin Islands, a large geographic region was sampled including much of the Gulf of Mexico and tropical Atlantic Ocean. Observations are reported for light-absorbing carbon aerosol (mainly black carbon, BC) primarily using a single particle soot photometer (SP2). The SP2 employs single-particle laser-induced incandescence to provide a mass-specific measurement not subject to scattering interference that is optimal for the low concentration environments like those encountered during GRIP. BC mass concentrations, 100-500 nm size distributions, and mixing state (i.e. coating thickness of scattering material) are presented. Total and sub-micron aerosol absorption coefficients (principally from BC and dust aerosol) are reported using a particle soot absorption photometer (PSAP) along with comparisons with calculated absorption coefficients derived from SP2 observations in various conditions. In addition, dust aerosol is specifically identified using optical and

  17. Uncertainties of aerosol retrieval from neglecting non-sphericity of dust aerosols

    NASA Astrophysics Data System (ADS)

    Li, Chi; Xue, Yong; Yang, Leiku; Guang, Jie

    2013-04-01

    The Mie theory is conventionally applied to calculate aerosol optical properties in satellite remote sensing applications, while dust aerosols cannot be well modeled by the Mie calculation for their non-sphericity. It has been cited in Mishchenko et al. (1995; 1997) that neglecting non-sphericity can severely influence aerosol optical depth (AOD, ?) retrieval in case of dust aerosols because of large difference of phase functions under spherical and non-spherical assumptions, whereas this uncertainty has not been thoroughly studied. This paper aims at a better understanding of uncertainties on AOD retrieval caused by aerosol non-sphericity. A dust aerosol model with known refractive index and size distribution is generated from long-term AERONET observations since 1999 over China. Then aerosol optical properties, such as the extinction, phase function, single scattering albedo (SSA) are calculated respectively in the assumption of spherical and non-spherical aerosols. Mie calculation is carried out for spherical assumption, meanwhile for non-spherical aerosol modeling, we adopt the pre-calculated scattering kernels and software package presented by Dubovik et al. (2002; 2006), which describes dust as a shape mixture of randomly oriented polydisperse spheroids. Consequently we generate two lookup tables (LUTspheric and LUTspheroid) from simulated satellite received reflectance at top of atmosphere (TOA) under varieties of observing conditions and aerosol loadings using Second Simulation of a Satellite Signal in the Solar Spectrum - Vector (6SV) code. All the simulations are made at 550 nm, and for simplicity the Lambertian surface is assumed. Using the obtained LUTs we examine the differences of TOA reflectance (Δ?TOA = ?spheric - ?spheroid) under different surface reflectance and aerosol loadings. Afterwards AOD is retrieved using LUTspheric from the simulated TOA reflectance by LUTspheroid in order to detect the retrieval errors (Δ? = ?retreived -?input) induced

  18. Estimation of global anthropogenic dust aerosol using CALIOP satellite

    NASA Astrophysics Data System (ADS)

    Chen, B.; Huang, J.; Liu, J.

    2014-12-01

    Anthropogenic dust aerosols are those produced by human activity, which mainly come from cropland, pasture, and urban in this paper. Because understanding of the emissions of anthropogenic dust is still very limited, a new technique for separating anthropogenic dust from natural dustusing CALIPSO dust and planetary boundary layer height retrievalsalong with a land use dataset is introduced. Using this technique, the global distribution of dust is analyzed and the relative contribution of anthropogenic and natural dust sources to regional and global emissions are estimated. Local anthropogenic dust aerosol due to human activity, such as agriculture, industrial activity, transportation, and overgrazing, accounts for about 22.3% of the global continentaldust load. Of these anthropogenic dust aerosols, more than 52.5% come from semi-arid and semi-wet regions. On the whole, anthropogenic dust emissions from East China and India are higher than other regions.

  19. Impact of Radiatively Interactive Dust Aerosols on Dust Transport and Mobilization in the NASA Goddard Earth Observing System (GEOS-5) Earth Model

    NASA Astrophysics Data System (ADS)

    Colarco, P. R.; Rocha Lima, A.; Darmenov, A.; Bloecker, C.

    2017-12-01

    Mineral dust aerosols scatter and absorb solar and infrared radiation, impacting the energy budget of the Earth system which in turns feeds back on the dynamical processes responsible for mobilization of dust in the first place. In previous work with radiatively interactive aerosols in the NASA Goddard Earth Observing System global model (GEOS-5) we found a positive feedback between dust absorption and emissions. Emissions were the largest for the highest shortwave absorption considered, which additionally produced simulated dust transport in the best agreement with observations. The positive feedback found was in contrast to other modeling studies which instead found a negative feedback, where the impact of dust absorption was to stabilize the surface levels of the atmosphere and so reduce wind speeds. A key difference between our model and other models was that in GEOS-5 we simulated generally larger dust particles, with correspondingly larger infrared absorption that led to a pronounced difference in the diurnal cycle of dust emissions versus simulations where these long wave effects were not considered. In this paper we seek to resolve discrepancies between our previous simulations and those of other modeling groups. We revisit the question of dust radiative feedback on emissions with a recent version of the GEOS-5 system running at a higher spatial resolution and including updates to the parameterizations for dust mobilization, initial dust particle size distribution, loss processes, and radiative transfer, and identify key uncertainties that remain based on dust optical property assumptions.

  20. Classification of Dust Days by Satellite Remotely Sensed Aerosol Products

    NASA Technical Reports Server (NTRS)

    Sorek-Hammer, M.; Cohen, A.; Levy, Robert C.; Ziv, B.; Broday, D. M.

    2013-01-01

    Considerable progress in satellite remote sensing (SRS) of dust particles has been seen in the last decade. From an environmental health perspective, such an event detection, after linking it to ground particulate matter (PM) concentrations, can proxy acute exposure to respirable particles of certain properties (i.e. size, composition, and toxicity). Being affected considerably by atmospheric dust, previous studies in the Eastern Mediterranean, and in Israel in particular, have focused on mechanistic and synoptic prediction, classification, and characterization of dust events. In particular, a scheme for identifying dust days (DD) in Israel based on ground PM10 (particulate matter of size smaller than 10 nm) measurements has been suggested, which has been validated by compositional analysis. This scheme requires information regarding ground PM10 levels, which is naturally limited in places with sparse ground-monitoring coverage. In such cases, SRS may be an efficient and cost-effective alternative to ground measurements. This work demonstrates a new model for identifying DD and non-DD (NDD) over Israel based on an integration of aerosol products from different satellite platforms (Moderate Resolution Imaging Spectroradiometer (MODIS) and Ozone Monitoring Instrument (OMI)). Analysis of ground-monitoring data from 2007 to 2008 in southern Israel revealed 67 DD, with more than 88 percent occurring during winter and spring. A Classification and Regression Tree (CART) model that was applied to a database containing ground monitoring (the dependent variable) and SRS aerosol product (the independent variables) records revealed an optimal set of binary variables for the identification of DD. These variables are combinations of the following primary variables: the calendar month, ground-level relative humidity (RH), the aerosol optical depth (AOD) from MODIS, and the aerosol absorbing index (AAI) from OMI. A logistic regression that uses these variables, coded as binary

  1. Identifying Aerosol Type/Mixture from Aerosol Absorption Properties Using AERONET

    NASA Technical Reports Server (NTRS)

    Giles, D. M.; Holben, B. N.; Eck, T. F.; Sinyuk, A.; Dickerson, R. R.; Thompson, A. M.; Slutsker, I.; Li, Z.; Tripathi, S. N.; Singh, R. P.; hide

    2010-01-01

    Aerosols are generated in the atmosphere through anthropogenic and natural mechanisms. These sources have signatures in the aerosol optical and microphysical properties that can be used to identify the aerosol type/mixture. Spectral aerosol absorption information (absorption Angstrom exponent; AAE) used in conjunction with the particle size parameterization (extinction Angstrom exponent; EAE) can only identify the dominant absorbing aerosol type in the sample volume (e.g., black carbon vs. iron oxides in dust). This AAE/EAE relationship can be expanded to also identify non-absorbing aerosol types/mixtures by applying an absorption weighting. This new relationship provides improved aerosol type distinction when the magnitude of absorption is not equal (e.g, black carbon vs. sulfates). The Aerosol Robotic Network (AERONET) data provide spectral aerosol optical depth and single scattering albedo - key parameters used to determine EAE and AAE. The proposed aerosol type/mixture relationship is demonstrated using the long-term data archive acquired at AERONET sites within various source regions. The preliminary analysis has found that dust, sulfate, organic carbon, and black carbon aerosol types/mixtures can be determined from this AAE/EAE relationship when applying the absorption weighting for each available wavelength (Le., 440, 675, 870nm). Large, non-spherical dust particles absorb in the shorter wavelengths and the application of 440nm wavelength absorption weighting produced the best particle type definition. Sulfate particles scatter light efficiently and organic carbon particles are small near the source and aggregate over time to form larger less absorbing particles. Both sulfates and organic carbon showed generally better definition using the 870nm wavelength absorption weighting. Black carbon generation results from varying combustion rates from a number of sources including industrial processes and biomass burning. Cases with primarily black carbon showed

  2. Quasar 2175 Å dust absorbers - I. Metallicity, depletion pattern and kinematics

    NASA Astrophysics Data System (ADS)

    Ma, Jingzhe; Ge, Jian; Zhao, Yinan; Prochaska, J. Xavier; Zhang, Shaohua; Ji, Tuo; Schneider, Donald P.

    2017-12-01

    We present 13 new 2175 Å dust absorbers at zabs = 1.0-2.2 towards background quasars from the Sloan Digital Sky Survey. These absorbers are examined in detail using data from the Echelle Spectrograph and Imager (ESI) on the Keck II telescope. Many low-ionization lines including Fe II, Zn II, Mg II, Si II, Al II, Ni II, Mn II, Cr II, Ti II and Ca II are present in the same absorber that gives rise to the 2175 Å bump. The relative metal abundances (with respect to Zn) demonstrate that the depletion patterns of our 2175 Å dust absorbers resemble that of the Milky Way clouds although some are disc-like and some are halo-like. The 2175 Å dust absorbers have significantly higher depletion levels compared to literature damped Lyman α absorbers (DLAs) and sub-DLAs. The dust depletion level indicator [Fe/Zn] tends to anticorrelate with bump strengths. The velocity profiles from the Keck/ESI spectra also provide kinematical information on the dust absorbers. The dust absorbers are found to have multiple velocity components with velocity widths extending from ∼100 to ∼600 km s-1, which are larger than those of most DLAs and sub-DLAs. Assuming the velocity width is a reliable tracer of stellar mass, the host galaxies of 2175 Å dust absorbers are expected to be more massive than DLA/sub-DLA hosts. Not all of the 2175 Å dust absorbers are intervening systems towards background quasars. The absorbers towards quasars J1006+1538 and J1047+3423 are proximate systems that could be associated with the quasar itself or the host galaxy.

  3. Influence of mineral dust transport on the chemical composition and physical properties of the Eastern Mediterranean aerosol

    NASA Astrophysics Data System (ADS)

    Koçak, M.; Theodosi, C.; Zarmpas, P.; Séguret, M. J. M.; Herut, B.; Kallos, G.; Mihalopoulos, N.; Kubilay, N.; Nimmo, M.

    2012-09-01

    Bulk aerosol samples were collected from three different coastal rural sites located around the Eastern Mediterranean, (i) Erdemli (ER), Turkey, (ii) Heraklion (HR), Crete, Greece, and (iii) Tel Shikmona (TS), Israel, during two distinct mineral dust periods (October, 2007 and April, 2008) in order to explore the temporal and geographical variability in the aerosol chemical composition. Samples were analyzed for trace elements (Al, Fe, Mn, Ca, Cr, Zn, Cu, V, Ni, Cd, Pb) and water-soluble ions (Cl-, NO3-, SO42-, C2O42-, Na+, NH4+, K+, Mg2+ and Ca2+). The dust events were categorized on the basis of Al concentrations >1000 ng m-3, SKIRON dust forecast model and 3-day back trajectories into three groups namely, Middle East, Mixed and Saharan desert. ER and TS were substantially affected by dust events originating from the Middle East, particularly in October, whilst HR was not influenced by dust transport from the Middle East. Higher AOT values were particularly associated with higher Al concentrations. Contrary to the highest Al concentration: 6300 ng m-3, TS showed relatively lower AI and AOT. Al concentrations at ER were similar for October and April, whilst OMI-AI and AOT values were ˜2 times higher in April. This might be attributed to the weak sensitivity of the TOMS instrument to absorbing aerosols near the ground and optical difference between Middle East and Saharan desert dusts. The lowest enhancement of anthropogenic aerosol species was observed at HR during dust events (nssSO42-/nssCa2+ ˜ 0.13). These species were particularly enhanced when mineral dust arrived at sites after passing through populated and industrialized urban areas.

  4. Radiative forcing and rapid adjustment of absorbing aerosols in the Pearl River Delta Region of China

    NASA Astrophysics Data System (ADS)

    Liu, Z.; Yim, S. H. L.; Lau, G.

    2016-12-01

    offsets part of the aerosol instantaneous negative radiation forcing, especially at TOA and SFC. The only absorbing aerosol species included in the test is BC. If absorption effects of dust and BrC are considered, the contribution of instantaneous radiative forcing and rapid adjustment may change.

  5. Interactive Soil Dust Aerosol Model in the GISS GCM. Part 1; Sensitivity of the Soil Dust Cycle to Radiative Properties of Soil Dust Aerosols

    NASA Technical Reports Server (NTRS)

    Perlwitz, Jan; Tegen, Ina; Miller, Ron L.

    2000-01-01

    The sensitivity of the soil dust aerosol cycle to the radiative forcing by soil dust aerosols is studied. Four experiments with the NASA/GISS atmospheric general circulation model, which includes a soil dust aerosol model, are compared, all using a prescribed climatological sea surface temperature as lower boundary condition. In one experiment, dust is included as dynamic tracer only (without interacting with radiation), whereas dust interacts with radiation in the other simulations. Although the single scattering albedo of dust particles is prescribed to be globally uniform in the experiments with radiatively active dust, a different single scattering albedo is used in those experiments to estimate whether regional variations in dust optical properties, corresponding to variations in mineralogical composition among different source regions, are important for the soil dust cycle and the climate state. On a global scale, the radiative forcing by dust generally causes a reduction in the atmospheric dust load corresponding to a decreased dust source flux. That is, there is a negative feedback in the climate system due to the radiative effect of dust. The dust source flux and its changes were analyzed in more detail for the main dust source regions. This analysis shows that the reduction varies both with the season and with the single scattering albedo of the dust particles. By examining the correlation with the surface wind, it was found that the dust emission from the Saharan/Sahelian source region and from the Arabian peninsula, along with the sensitivity of the emission to the single scattering albedo of dust particles, are related to large scale circulation patterns, in particular to the trade winds during Northern Hemisphere winter and to the Indian monsoon circulation during summer. In the other regions, such relations to the large scale circulation were not found. There, the dependence of dust deflation to radiative forcing by dust particles is probably

  6. Global Distribution of Dust, Smoke, Volcanic Ash, and Pollutant Aerosols Seen from Space

    NASA Technical Reports Server (NTRS)

    Herman, Jay R.; Hsu, Christina; Krotkov, Nickolay; Torres, Omar

    1998-01-01

    New technique for observing aerosols from space, using ultraviolet (UV) wavelengths, have been developed during the past three years. The chief benefit from observing aerosols in the UV is that they are easily visible over both land and water. While there is presently more than one satellite that can observe aerosols in the UV, only Total Ozone Mapping Spectrometer (TOMS) has a long-term record (since 1979) and adequate spatial resolutions (50 to 100 km) to observe the seasonal and interannual variations, and to locate some of the land sources of dust, smoke, volcanic ash and sulfate pollutants. The data has been assembled into daily images of the atmospheric aerosol loading in terms of optical depth and UV transmittance. For the major sources of aerosols, it is common for at least 50% of the total UV to be absorbed underneath aerosol plumes. This is particularly true for the spectacular smoke plumes originating from the recent Indonesian and Mexican fires, as well as under the huge African dust plumes. The sulfate pollutants are mostly present in the Northern Hemisphere and are associated with regions of high industrial activity. The location and seasonal dependence of these aerosol plumes over Europe and North America will be contrasted with the relatively clean Southern Hemisphere. Because of the success of this technique, it has formed the basis for a new generation of space-borne aerosol detection instruments. These new instruments combine the UV observations with the more traditional visible-wavelength data to obtain a more comprehensive characterization of aerosols that is possible with either UV or visible techniques by themselves.

  7. MGS TES Measurements of Dust and Ice Aerosol Behaviors

    NASA Astrophysics Data System (ADS)

    Clancy, R. T.; Wolff, M. J.; Christensen, P. R.

    2000-10-01

    The Thermal Emission Spectrometer (TES, Christensen et al., Science, v279, 1692-1697, 1998) on board the Mars Global Surveyor obtains simultaneous solar band and thermal IR spectral emission-phase-function (EPF) observations with global spatial coverage and continuous seasonal sampling. These measurements allow the first comprehensive study of the coupled visible scattering and thermal IR absorption properties of Mars atmospheric aerosols, a fundamental requirement towards defining opacities, particle sizes, and particle shapes for separable dust and water ice aerosol components. Furthermore, TES limb sounding at solar band and IR wavelengths may be analyzed in the context of these EPF column determinations to constrain the distinctive vertical profile behaviors of dust and ice clouds. We present initial radiative transfer analyses of TES visible and IR EPFs, which indicate surprisingly complex dust and ice aerosol behaviors over all latitudes and seasons. Distinctive backscattering peaks of variable intensity are observed for several types of water ice clouds, along with evidence for ice-coated dust aerosols. We will present a broad spatial and temporal sampling of solar band and spectral IR results for Mars atmospheric ice and dust aerosols observed over the 1998-2000 period. This research is supported by the MGS Participating Scientist and MED Science Data Analysis programs.

  8. Dust radiative effect over Europe, Mediterranean, Sahara and Middle East from a radiative transfer model using BSC-DREAM8b aerosol optical data

    NASA Astrophysics Data System (ADS)

    Papadimas, Christos; Gkikas, Antonis; Hatzianastassiou, Nikos; Matsoukas, Christos; Kazadzis, Stelios; Basart, Sara; Baldasano, Jose; Vardavas, Ilias

    2013-04-01

    The arid regions of Saharan desert and Middle East are the world's major dust sources. However, dust particles from these areas are transported to nearby regions, through favourable synoptic conditions, even reaching remote locations in Europe or in the Arctic. This transport is very important in numerous aspects. One of its most important effects is on the radiation budget, and more specifically on solar radiation, through the aerosol direct radiative effect (DRE). Previous studies have shown that this effect is great under dust load conditions. Therefore, it is very important to simulate dust transport processes and associated radiative effects. The simulation of dust production, transport and removal is done by numerical models, which however have their own limitations as to the consideration of physical and dynamical processes as well as their initial conditions. On the other hand, the computation of dust DRE is ideally done with radiative transfer models (RTMs), which however imply uncertainties associated with the input aerosol optical properties. The most important aerosol optical properties used in RTMs and climate models are aerosol optical depth (AOD), single scattering albedo (SSA) and asymmetry parameter (AP). The main target of the present study is to reduce the uncertainties of dust DRE by using a detailed spectral RTM and an acknowledged regional and meso-scale model describing the distribution of dust. The combined use of these tools is applied to the region covering the deserts of Sahara, Arabian Peninsula and Middle East, and the neighbouring Mediterranean basin and European continent (extending from 15°N to 60°N and from 21°W to 54°E). The computations are performed on a monthly mean basis, refer to the 11-year period 2000-2010, and quantify the effects of dust on the reflected solar radiation at the top of atmosphere (DRETOA), on the absorbed solar radiation within the atmosphere (DREatmab), and on the downwelling and absorbed solar

  9. Ice Nucleation Activity of Various Agricultural Soil Dust Aerosol Particles

    NASA Astrophysics Data System (ADS)

    Schiebel, Thea; Höhler, Kristina; Funk, Roger; Hill, Thomas C. J.; Levin, Ezra J. T.; Nadolny, Jens; Steinke, Isabelle; Suski, Kaitlyn J.; Ullrich, Romy; Wagner, Robert; Weber, Ines; DeMott, Paul J.; Möhler, Ottmar

    2016-04-01

    Recent investigations at the cloud simulation chamber AIDA (Aerosol Interactions and Dynamics in the Atmosphere) suggest that agricultural soil dust has an ice nucleation ability that is enhanced up to a factor of 10 compared to desert dust, especially at temperatures above -26 °C (Steinke et al., in preparation for submission). This enhancement might be caused by the contribution of very ice-active biological particles. In addition, soil dust aerosol particles often contain a considerably higher amount of organic matter compared to desert dust particles. To test agricultural soil dust as a source of ice nucleating particles, especially for ice formation in warm clouds, we conducted a series of laboratory measurements with different soil dust samples to extend the existing AIDA dataset. The AIDA has a volume of 84 m3 and operates under atmospherically relevant conditions over wide ranges of temperature, pressure and humidity. By controlled adiabatic expansions, the ascent of an air parcel in the troposphere can be simulated. As a supplement to the AIDA facility, we use the INKA (Ice Nucleation Instrument of the KArlsruhe Institute of Technology) continuous flow diffusion chamber based on the design by Rogers (1988) to expose the sampled aerosol particles to a continuously increasing saturation ratio by keeping the aerosol temperature constant. For our experiments, soil dust was dry dispersed into the AIDA vessel. First, fast saturation ratio scans at different temperatures were performed with INKA, sampling soil dust aerosol particles directly from the AIDA vessel. Then, we conducted the AIDA expansion experiment starting at a preset temperature. The combination of these two different methods provides a robust data set on the temperature-dependent ice activity of various agriculture soil dust aerosol particles with a special focus on relatively high temperatures. In addition, to extend the data set, we investigated the role of biological and organic matter in more

  10. Aerosol transport over the western Mediterranean basin: Evidence of the contribution of fine particles to desert dust plumes over Alborán Island

    NASA Astrophysics Data System (ADS)

    Valenzuela, A.; Olmo, F. J.; Lyamani, H.; Granados-Muñoz, M. J.; Antón, M.; Guerrero-Rascado, J. L.; Quirantes, A.; Toledano, C.; Perez-Ramírez, D.; Alados-Arboledas, L.

    2014-12-01

    Eight months (June 2011 to January 2012) of aerosol property data were obtained at the remote site of Alborán Island (35.95°N, 3.03°W) in the western Mediterranean basin. The aim of this work is to assess the aerosol properties according to air mass origin and transport over this remote station with a special focus on air mass transport from North Africa. For air masses coming from North Africa, different aerosol properties showed strong contributions from mineral dust lifted from desert areas. Nevertheless, during these desert dust intrusions, some atmospheric aerosol properties are clearly different from pure mineral dust particles. Thus, Angström exponent α(440-870) presents larger values than those reported for pure desert dust measured close to dust source regions. These results combine with α(440, 670) - α(670, 870) ≥ 0.1 and low single scattering albedo (ω(λ)) values, especially at the largest wavelengths. Most of the desert dust intrusions over Alborán can be described as a mixture of dust and anthropogenic particles. The analyses support that our results apply to North Africa desert dust air masses transported from different source areas. Therefore, our results indicate a significant contribution of fine absorbing particles during desert dust intrusions over Alborán arriving from different source regions. The aerosol optical depth data retrieved from Sun photometer measurements have been used to check Moderate Resolution Imaging Spectroradiometer retrievals, and they show reasonable agreement, especially for North African air masses.

  11. Disturbance of light-absorbing aerosols on the albedo in a winter snowpack of Central Tibet.

    PubMed

    Ming, Jing; Wang, Pengling; Zhao, Shuyu; Chen, Pengfei

    2013-08-01

    A field observation on the albedo of the snowpack in Central Tibet was conducted in the Nam Co region in the winter of 2011. Snow properties, including grain size and density, were measured in the field, and surface-layer snow samples (down to 5 cm) were collected. The average concentrations of black carbon and dust were 72 ppbm (close to that in the glaciers of Mt. Nyainqentanglha) and 120 ppmm, respectively. Inverse trends were found to exist between the albedo of the snowpack and light-absorbing aerosols (LAAs) as well as grain size growth. Modeling showed that black carbon, dust, and grain growth in the winter snowpack can reduce the broadband albedo by 11%, 28%, and 61%, respectively.

  12. Integrated approach towards understanding interactions of mineral dust aerosol with warm clouds

    NASA Astrophysics Data System (ADS)

    Kumar, Prashant

    2011-12-01

    Mineral dust is ubiquitous in the atmosphere and represents a dominant type of particulate matter by mass. Dust particles can serve as cloud condensation nuclei (CCN), giant CCN (GCCN), or ice nuclei (IN), thereby, affecting cloud microphysics, albedo, and lifetime. Despite its well-recognized importance, assessments of dust impacts on clouds and climate remain highly uncertain. This thesis addresses the role of dust as CCN and GCCN with the goal of improving our understanding of dust-warm cloud interactions and their representation in climate models. Most studies to date focus on the soluble fraction of aerosol particles when describing cloud droplet nucleation, and overlook the interactions of the hydrophilic insoluble fraction with water vapor. A new approach to include such interactions (expressed by the process of water vapor adsorption) is explored, by combining multilayer Frenkel-Halsey-Hill (FHH) physical adsorption isotherm and curvature (Kelvin) effects. The importance of adsorption activation theory (FHH-AT) is corroborated by measurements of CCN activity of mineral aerosols generated from clays, calcite, quartz, and desert soil samples from Northern Africa, East Asia/China, and Northern America. A new aerosol generation setup for CCN measurements was developed based on a dry generation technique capable of reproducing natural dust aerosol emission. Based on the dependence of critical supersaturation with particle dry diameter, it is found that the FHH-AT is a better framework for describing fresh (and unprocessed) dust CCN activity than the classical Kohler theory (KT). Ion Chromatography (IC) measurements performed on fresh regional dust samples indicate negligible soluble fraction, and support that water vapor adsorption is the prime source of CCN activity in the dust. CCN measurements with the commonly used wet generated mineral aerosol (from atomization of a dust aqueous suspension) are also carried out. Results indicate that the method is subject

  13. Aircraft and ground measurements of dust aerosols over the west African coast in summer 2015 during ICE-D and AER-D

    NASA Astrophysics Data System (ADS)

    Liu, Dantong; Taylor, Jonathan W.; Crosier, Jonathan; Marsden, Nicholas; Bower, Keith N.; Lloyd, Gary; Ryder, Claire L.; Brooke, Jennifer K.; Cotton, Richard; Marenco, Franco; Blyth, Alan; Cui, Zhiqiang; Estelles, Victor; Gallagher, Martin; Coe, Hugh; Choularton, Tom W.

    2018-03-01

    During the summertime, dust from the Sahara can be efficiently transported westwards within the Saharan air layer (SAL). This can lead to high aerosol loadings being observed above a relatively clean marine boundary layer (MBL) in the tropical Atlantic Ocean. These dust layers can impart significant radiative effects through strong visible and IR light absorption and scattering, and can also have indirect impacts by altering cloud properties. The processing of the dust aerosol can result in changes in both direct and indirect radiative effects, leading to significant uncertainty in climate prediction in this region. During August 2015, measurements of aerosol and cloud properties were conducted off the coast of west Africa as part of the Ice in Cloud Experiment - Dust (ICE-D) and AERosol properties - Dust (AER-D) campaigns. Observations were obtained over a 4-week period using the UK Facility for Atmospheric Airborne Measurements (FAAM) BAe 146 aircraft based on Santiago Island, Cabo Verde. Ground-based observations were collected from Praia (14°57' N, 23°29' W; 100 m a.s.l.), also located on Santiago Island. The dust in the SAL was mostly sampled in situ at altitudes of 2-4 km, and the potential dust age was estimated by backward trajectory analysis. The particle mass concentration (at diameter d = 0.1-20 µm) decreased with transport time. Mean effective diameter (Deff) for supermicron SAL dust (d = 1-20 µm) was found to be 5-6 µm regardless of dust age, whereas submicron Deff (d = 0.1-1 µm) showed a decreasing trend with longer transport. For the first time, an airborne laser-induced incandescence instrument (the single particle soot photometer - SP2) was deployed to measure the hematite content of dust. For the Sahel-influenced dust in the SAL, the observed hematite mass fraction of dust (FHm) was found to be anti-correlated with the single scattering albedo (SSA, λ = 550 nm, for particles d < 2.5 µm); as potential dust age increased from 2 to 7 days

  14. Radiative absorption enhancement of dust mixed with anthropogenic pollution over East Asia

    NASA Astrophysics Data System (ADS)

    Tian, Pengfei; Zhang, Lei; Ma, Jianmin; Tang, Kai; Xu, Lili; Wang, Yuan; Cao, Xianjie; Liang, Jiening; Ji, Yuemeng; Jiang, Jonathan H.; Yung, Yuk L.; Zhang, Renyi

    2018-06-01

    The particle mixing state plays a significant yet poorly quantified role in aerosol radiative forcing, especially for the mixing of dust (mineral absorbing) and anthropogenic pollution (black carbon absorbing) over East Asia. We have investigated the absorption enhancement of mixed-type aerosols over East Asia by using the Aerosol Robotic Network observations and radiative transfer model calculations. The mixed-type aerosols exhibit significantly enhanced absorbing ability than the corresponding unmixed dust and anthropogenic aerosols, as revealed in the spectral behavior of absorbing aerosol optical depth, single scattering albedo, and imaginary refractive index. The aerosol radiative efficiencies for the dust, mixed-type, and anthropogenic aerosols are -101.0, -112.9, and -98.3 Wm-2 τ-1 at the bottom of the atmosphere (BOA); -42.3, -22.5, and -39.8 Wm-2 τ-1 at the top of the atmosphere (TOA); and 58.7, 90.3, and 58.5 Wm-2 τ-1 in the atmosphere (ATM), respectively. The BOA cooling and ATM heating efficiencies of the mixed-type aerosols are significantly higher than those of the unmixed aerosol types over the East Asia region, resulting in atmospheric stabilization. In addition, the mixed-type aerosols correspond to a lower TOA cooling efficiency, indicating that the cooling effect by the corresponding individual aerosol components is partially counteracted. We conclude that the interaction between dust and anthropogenic pollution not only represents a viable aerosol formation pathway but also results in unfavorable dispersion conditions, both exacerbating the regional air pollution in East Asia. Our results highlight the necessity to accurately account for the mixing state of aerosols in atmospheric models over East Asia in order to better understand the formation mechanism for regional air pollution and to assess its impacts on human health, weather, and climate.

  15. A 20-year simulated climatology of global dust aerosol deposition.

    PubMed

    Zheng, Yu; Zhao, Tianliang; Che, Huizheng; Liu, Yu; Han, Yongxiang; Liu, Chong; Xiong, Jie; Liu, Jianhui; Zhou, Yike

    2016-07-01

    Based on a 20-year (1991-2010) simulation of dust aerosol deposition with the global climate model CAM5.1 (Community Atmosphere Model, version 5.1), the spatial and temporal variations of dust aerosol deposition were analyzed using climate statistical methods. The results indicated that the annual amount of global dust aerosol deposition was approximately 1161±31Mt, with a decreasing trend, and its interannual variation range of 2.70% over 1991-2010. The 20-year average ratio of global dust dry to wet depositions was 1.12, with interannual variation of 2.24%, showing the quantity of dry deposition of dust aerosol was greater than dust wet deposition. High dry deposition was centered over continental deserts and surrounding regions, while wet deposition was a dominant deposition process over the North Atlantic, North Pacific and northern Indian Ocean. Furthermore, both dry and wet deposition presented a zonal distribution. To examine the regional changes of dust aerosol deposition on land and sea areas, we chose the North Atlantic, Eurasia, northern Indian Ocean, North Pacific and Australia to analyze the interannual and seasonal variations of dust deposition and dry-to-wet deposition ratio. The deposition amounts of each region showed interannual fluctuations with the largest variation range at around 26.96% in the northern Indian Ocean area, followed by the North Pacific (16.47%), Australia (9.76%), North Atlantic (9.43%) and Eurasia (6.03%). The northern Indian Ocean also had the greatest amplitude of interannual variation in dry-to-wet deposition ratio, at 22.41%, followed by the North Atlantic (9.69%), Australia (6.82%), North Pacific (6.31%) and Eurasia (4.36%). Dust aerosol presented a seasonal cycle, with typically strong deposition in spring and summer and weak deposition in autumn and winter. The dust deposition over the northern Indian Ocean exhibited the greatest seasonal change range at about 118.00%, while the North Atlantic showed the lowest seasonal

  16. Synergy of Satellite-Surface Observations for Studying the Properties of Absorbing Aerosols in Asia

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee

    2010-01-01

    Through interaction with clouds and alteration of the Earth's radiation budget, atmospheric aerosols significantly influence our weather and climate. Monsoon rainfalls, for example, sustain the livelihood of more than half of the world's population. Thus, understanding the mechanism that drives the water cycle and freshwater distribution is high-lighted as one of the major near-term goals in NASA's Earth Science Enterprise Strategy. Every cloud droplet/ice-crystal that serves as an essential element in portraying water cycle and distributing freshwater contains atmospheric aerosols at its core. In addition, the spatial and temporal variability of atmospheric aerosol properties is complex due to their dynamic nature. In fact, the predictability of the tropical climate system is much reduced during the boreal spring, which is associated with the peak season of biomass burning activities and regional/long-range transport of dust aerosols. Therefore, to accurately assess the impact of absorbing aerosols on regional-to-global climate requires not only modeling efforts but also continuous observations from satellites, aircraft, networks of ground-based instruments and dedicated field experiments. Since 1997 NASA has been successfully launching a series of satellites the Earth Observing System - to intensively study, and gain a better understanding of, the Earth as an integrated system. Through participation in many satellite remote-sensing/retrieval and validation projects over the years, we have gradually developed and refined the SMART (Surface-sensing Measurements for Atmospheric Radiative Transfer) and COMMIT (Chemical, Optical & Microphysical Measurements of In-situ Troposphere) mobile observatories, a suite of surface remote sensing and in-situ instruments that proved to be vital in providing high temporal measurements, which complement the satellite observations. In this talk, we will present SMART-COMMIT which has played key roles, serving as network or supersite

  17. Changes in Stratiform Clouds of Mesoscale Convective Complex Introduced by Dust Aerosols

    NASA Technical Reports Server (NTRS)

    Lin, B.; Min, Q.-L.; Li, R.

    2010-01-01

    Aerosols influence the earth s climate through direct, indirect, and semi-direct effects. There are large uncertainties in quantifying these effects due to limited measurements and observations of aerosol-cloud-precipitation interactions. As a major terrestrial source of atmospheric aerosols, dusts may serve as a significant climate forcing for the changing climate because of its effect on solar and thermal radiation as well as on clouds and precipitation processes. Latest satellites measurements enable us to determine dust aerosol loadings and cloud distributions and can potentially be used to reduce the uncertainties in the estimations of aerosol effects on climate. This study uses sensors on various satellites to investigate the impact of mineral dust on cloud microphysical and precipitation processes in mesoscale convective complex (MCC). A trans-Atlantic dust outbreak of Saharan origin occurring in early March 2004 is considered. For the observed MCCs under a given convective strength, small hydrometeors were found more prevalent in the dusty stratiform regions than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust regions, particularly at altitudes where heterogeneous nucleation of mineral dust prevails, further supports the observed changes of clouds and precipitation. The consequences of the microphysical effects of the dust aerosols were to shift the size spectrum of precipitation-sized hydrometeors from heavy precipitation to light precipitation and ultimately to suppress precipitation and increase the lifecycle of cloud systems, especially over stratiform areas.

  18. Solar Spectral Radiative Forcing Due to Dust Aerosol During the Puerto Rico Dust Experiment

    NASA Technical Reports Server (NTRS)

    Pilewskie, P.; Bergstrom, R.; Rabbette, M.; Livingston, J.; Russell, P.; Gore, Warren J. (Technical Monitor)

    2000-01-01

    During the Puerto Rico Dust Experiment (PRIDE) upwelling and downwelling solar spectral irradiance was measured on board the SPAWAR Navajo and downwelling solar spectral flux was measured at a surface site using the NASA Ames Solar Spectral Flux Radiometer. These data will be used to determine the net solar radiative forcing of dust aerosol and to quantify the solar spectral radiative energy budget in the presence of elevated aerosol loading. We will assess the variability in spectral irradiance using formal principal component analysis procedures and relate the radiative variability to aerosol microphysical properties. Finally, we will characterize the sea surface reflectance to improve aerosol optical depth retrievals from the AVHRR satellite and to validate SeaWiFS ocean color products.

  19. Exploring the Longwave Radiative Effects of Dust Aerosols

    NASA Technical Reports Server (NTRS)

    Hansell, Richard A., Jr.

    2012-01-01

    Dust aerosols not only affect air quality and visibility where they pose a significant health and safety risk, but they can also play a role in modulating the energy balance of the Earth-atmosphere system by directly interacting with local radiative fields. Consequently, dust aerosols can impact regional climate patterns such as changes in precipitation and the evolution of the hydrological cycle. Assessing the direct effect of dust aerosols at the solar wavelengths is fairly straightforward due in part to the relatively large signal-to-noise ratio in broadband irradiance measurements. The longwave (LW) impacts, on the other hand, are rather difficult to ascertain since the measured dust signal level (10 Wm-2) is on the same order as the instrumental uncertainties. Moreover, compared to the shortwave (SW), limited experimental data on the LW optical properties of dust makes it a difficult challenge for constraining the LW impacts. Owing to the strong absorption features found in many terrestrial minerals (e.g., silicates and clays), the LW effects, although much smaller in magnitude compared to the SW, can still have a sizeable impact on the energetics of the Earth-atmosphere system, which can potentially trigger changes in the heat and moisture surface budgets, and dynamics of the atmosphere. The current endeavor is an integral part of an on-going research study to perform detailed assessments of dust direct aerosol radiative effects (DARE) using comprehensive global datasets from NASA Goddards mobile ground-based facility (cf. http://smartlabs.gsfc.nasa.gov/) during previous field experiments near key dust source regions. Here we examine and compare the results from two of these studies: the 2006 NASA African Monsoon Multidisciplinary Activities and the 2008 Asian Monsoon Years. The former study focused on transported Saharan dust at Sal Island (16.73N, 22.93W), Cape Verde along the west coast of Africa while the latter focused on Asian dust at Zhangye China (39

  20. Aethalometer multiple scattering correction Cref for mineral dust aerosols

    NASA Astrophysics Data System (ADS)

    Di Biagio, Claudia; Formenti, Paola; Cazaunau, Mathieu; Pangui, Edouard; Marchand, Nicolas; Doussin, Jean-François

    2017-08-01

    In this study we provide a first estimate of the Aethalometer multiple scattering correction Cref for mineral dust aerosols. Cref is an empirical constant used to correct the aerosol absorption coefficient measurements for the multiple scattering artefact of the Aethalometer; i.e. the filter fibres on which aerosols are deposited scatter light and this is miscounted as absorption. The Cref at 450 and 660 nm was obtained from the direct comparison of Aethalometer data (Magee Sci. AE31) with (i) the absorption coefficient calculated as the difference between the extinction and scattering coefficients measured by a Cavity Attenuated Phase Shift Extinction analyser (CAPS PMex) and a nephelometer respectively at 450 nm and (ii) the absorption coefficient from a MAAP (Multi-Angle Absorption Photometer) at 660 nm. Measurements were performed on seven dust aerosol samples generated in the laboratory by the mechanical shaking of natural parent soils issued from different source regions worldwide. The single scattering albedo (SSA) at 450 and 660 nm and the size distribution of the aerosols were also measured. Cref for mineral dust varies between 1.81 and 2.56 for a SSA of 0.85-0.96 at 450 nm and between 1.75 and 2.28 for a SSA of 0.98-0.99 at 660 nm. The calculated mean for dust is 2.09 (±0.22) at 450 nm and 1.92 (±0.17) at 660 nm. With this new Cref the dust absorption coefficient by the Aethalometer is about 2 % (450 nm) and 11 % (660 nm) higher than that obtained by using Cref = 2.14 at both 450 and 660 nm, as usually assumed in the literature. This difference induces a change of up to 3 % in the dust SSA at 660 nm. The Cref seems to be independent of the fine and coarse particle size fractions, and so the obtained Cref can be applied to dust both close to sources and following transport. Additional experiments performed with pure kaolinite minerals and polluted ambient aerosols indicate Cref of 2.49 (±0.02) and 2.32 (±0.01) at 450 and 660 nm (SSA = 0.96-0.97) for

  1. Vertical Structure of Aerosols and Mineral Dust Over the Bay of Bengal From Multisatellite Observations

    NASA Astrophysics Data System (ADS)

    Lakshmi, N. B.; Nair, Vijayakumar S.; Suresh Babu, S.

    2017-12-01

    The vertical distribution of aerosol and dust extinction coefficient over the Bay of Bengal is examined using the satellite observations (Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) and Moderate Resolution Imaging Spectroradiometer (MODIS)) for the period from 2006 to 2017. Distinct seasonal pattern is observed in the vertical structure of both aerosol and dust over the Bay of Bengal with an enhancement of 24% in the aerosol extinction above 1 km from winter (December, January and February) to premonsoon (March, April, and May). Significant contribution of dust is observed over the northern Bay of Bengal during premonsoon season where 22% of the total aerosol extinction is contributed by dust aerosols transported from the nearby continental regions. During winter, dust transport is found to be less significant with fractional contribution of 10%-13% to the total aerosol optical depth over the Bay of Bengal. MODIS-derived dust fraction (fine mode based) shows an overestimation up to twofold compared to CALIOP dust fraction (depolarization based), whereas the Goddard Chemistry Aerosol Radiation and Transport-simulated dust fraction underestimates the satellite-derived dust fractions over the Bay of Bengal. Though the long-term variation in dust aerosol showed a decreasing trend over the Bay of Bengal, the confidence level is insufficient in establishing the robustness of the observed trend. However, significant dust-induced heating is observed above the boundary layer during premonsoon season. This dust-induced elevated heating can affect the convection over the Bay of Bengal which will have implication on the monsoon dynamics over the Indian region.

  2. Water-soluble part of the aerosol in the dust storm season—evidence of the mixing between mineral and pollution aerosols

    NASA Astrophysics Data System (ADS)

    Wang, Ying; Zhuang, Guoshun; Sun, Yele; An, Zhisheng

    Six dust episodes were observed in Beijing in 2002. Both TSP (Total Suspended Particulate, particle size smaller than 100 μm) and PM 2.5 (particle size smaller than 2.5 μm) aerosol samples in these episodes were collected and their characteristics of water-soluble part were elaborated in demonstrating the mixing of mineral aerosol with pollution aerosol in the long-range transport of Asia aerosols with various sources and different paths. The dust storm peaked on 20 March, in which the highest concentrations of TSP and PM 2.5 were 10.9 and 1.4 mg m -3, respectively. The mass fraction of water-soluble part generally decreased with the increase of dust intensity. SO 42- contributed 38-70% to the total anions and Ca 2+ contributed 37-80% to the total cations, indicating that SO 42- and Ca 2+ were the most abundant anion and cation, respectively. The major ions of the water-soluble parts could be classified into three groups, i.e., the crust ions (Ca 2+, Na +, and Mg 2+), the pollution-crust ions (SO 42-, Cl -, and K +), and the pollution ions (NO 3-, NH 4+, NO 2-, and F -). Crust ions and pollution ions were the main ion fractions in super dust and non-dust days, respectively, whereas the pollution-crust ions were the main ion fractions in both dust days of various dust intensity and non-dust days, which demonstrated clearly that the mixing between mineral and pollution aerosols was ubiquitous during the dust seasons (even in the super dust storm days) although it was more obvious in those normal and weak dust episodes. The main chemical species of the water-soluble part of the aerosols were CaCO 3 in the super dust storm, CaSO 4 in the normal and the weak dust events, and NH 4NO 3 in the non-dust event days. The secondary transformation of sulfate and nitrate occurred on dust particles both during and after dust days provided the strong evidence of the mixing between mineral and pollution aerosols during the long-range transport of dust.

  3. A new stochastic algorithm for inversion of dust aerosol size distribution

    NASA Astrophysics Data System (ADS)

    Wang, Li; Li, Feng; Yang, Ma-ying

    2015-08-01

    Dust aerosol size distribution is an important source of information about atmospheric aerosols, and it can be determined from multiwavelength extinction measurements. This paper describes a stochastic inverse technique based on artificial bee colony (ABC) algorithm to invert the dust aerosol size distribution by light extinction method. The direct problems for the size distribution of water drop and dust particle, which are the main elements of atmospheric aerosols, are solved by the Mie theory and the Lambert-Beer Law in multispectral region. And then, the parameters of three widely used functions, i.e. the log normal distribution (L-N), the Junge distribution (J-J), and the normal distribution (N-N), which can provide the most useful representation of aerosol size distributions, are inversed by the ABC algorithm in the dependent model. Numerical results show that the ABC algorithm can be successfully applied to recover the aerosol size distribution with high feasibility and reliability even in the presence of random noise.

  4. Anomalies of the Asian Monsoon Induced by Aerosol Forcings

    NASA Technical Reports Server (NTRS)

    Lau, William K. M.; Kim, M. K.

    2004-01-01

    Impacts of aerosols on the Asian summer monsoon are studied using the NASA finite volume General Circulation Model (fvGCM), with radiative forcing derived from three-dimensional distributions of five aerosol species i.e., black carbon, organic carbon, soil dust, and sea salt from the Goddard Chemistry Aerosol Radiation and Transport Model (GOCART). Results show that absorbing aerosols, i.e., black carbon and dust, induce large-scale upper-level heating anomaly over the Tibetan Plateau in April and May, ushering in & early onset of the Indian summer monsoon. Absorbing aerosols also I i enhance lower-level heating and anomalous ascent over northern India, intensifying the Indian monsoon. Overall, the aerosol-induced large-scale surface' temperature cooling leads to a reduction of monsoon rainfall over the East Asia continent, and adjacent oceanic regions.

  5. Simulation of Asia Dust and Cloud Interaction Over Pacific Ocean During Pacdex

    NASA Astrophysics Data System (ADS)

    Long, X.; Huang, J.; Cheng, C.; Wang, W.

    2007-12-01

    The effect of dust plume on the Pacific cloud systems and the associated radiative forcing is an outstanding problem for understanding climate change. Many studies showing that dust aerosol might be a good absorber for solar radiation, at the same time dust aerosols could affect the cloud's formation and precipitation by its capability as cloud condensation nuclei (CCN) and ice forming nuclei (IFN). But the role of aerosols in clouds and precipitation is very complex. Simulation of interaction between cloud and dust aerosols requires recognition that the aerosol cloud system comprises coupled components of dynamics, aerosol and cloud microphysics, radiation processes. In this study, we investigated the interaction between dust aerosols and cloud with WRF which coupled with detailed cloud microphysics processes and dust process. The observed data of SACOL (Semi-Arid Climate and Environment Observatory of Lanzhou University) and PACDEX (Pacific Dust Experiment) is used as the initialization which include the vertical distributions and concentration of dust particles. Our results show that dust aerosol not only impacts cloud microphysical processes but also cloud microstructure; Dust aerosols can act as effective ice nuclei and intensify the ice-forming processes.

  6. Effect of Dust and Anthropogenic Aerosols on Columnar Aerosol Optical Properties over Darjeeling (2200 m asl), Eastern Himalayas, India

    PubMed Central

    Chatterjee, Abhijit; Ghosh, Sanjay K.; Adak, Anandamay; Singh, Ajay K.; Devara, Panuganti C. S.; Raha, Sibaji

    2012-01-01

    Background The loading of atmospheric particulate matter (aerosol) in the eastern Himalaya is mainly regulated by the locally generated anthropogenic aerosols from the biomass burning and by the aerosols transported from the distance sources. These different types of aerosol loading not only affect the aerosol chemistry but also produce consequent signature on the radiative properties of aerosol. Methodology/Principal Findings An extensive study has been made to study the seasonal variations in aerosol components of fine and coarse mode aerosols and black carbon along with the simultaneous measurements of aerosol optical depth on clear sky days over Darjeeling, a high altitude station (2200 masl) at eastern Himalayas during the year 2008. We observed a heavy loading of fine mode dust component (Ca2+) during pre-monsoon (Apr – May) which was higher by 162% than its annual mean whereas during winter (Dec – Feb), the loading of anthropogenic aerosol components mainly from biomass burning (fine mode SO4 2− and black carbon) were higher (76% for black carbon and 96% for fine mode SO4 2−) from their annual means. These high increases in dust aerosols during pre-monsoon and anthropogenic aerosols during winter enhanced the aerosol optical depth by 25 and 40%, respectively. We observed that for every 1% increase in anthropogenic aerosols, AOD increased by 0.55% during winter whereas for every 1% increase in dust aerosols, AOD increased by 0.46% during pre-monsoon. Conclusion/Significance The natural dust transport process (during pre-monsoon) plays as important a role in the radiation effects as the anthropogenic biomass burning (during winter) and their differential effects (rate of increase of the AOD with that of the aerosol concentration) are also very similar. This should be taken into account in proper modeling of the atmospheric environment over eastern Himalayas. PMID:22792264

  7. Effect of dust and anthropogenic aerosols on columnar aerosol optical properties over Darjeeling (2200 m asl), eastern Himalayas, India.

    PubMed

    Chatterjee, Abhijit; Ghosh, Sanjay K; Adak, Anandamay; Singh, Ajay K; Devara, Panuganti C S; Raha, Sibaji

    2012-01-01

    The loading of atmospheric particulate matter (aerosol) in the eastern Himalaya is mainly regulated by the locally generated anthropogenic aerosols from the biomass burning and by the aerosols transported from the distance sources. These different types of aerosol loading not only affect the aerosol chemistry but also produce consequent signature on the radiative properties of aerosol. An extensive study has been made to study the seasonal variations in aerosol components of fine and coarse mode aerosols and black carbon along with the simultaneous measurements of aerosol optical depth on clear sky days over Darjeeling, a high altitude station (2200 masl) at eastern Himalayas during the year 2008. We observed a heavy loading of fine mode dust component (Ca(2+)) during pre-monsoon (Apr-May) which was higher by 162% than its annual mean whereas during winter (Dec-Feb), the loading of anthropogenic aerosol components mainly from biomass burning (fine mode SO(4)(2-) and black carbon) were higher (76% for black carbon and 96% for fine mode SO(4)(2-)) from their annual means. These high increases in dust aerosols during pre-monsoon and anthropogenic aerosols during winter enhanced the aerosol optical depth by 25 and 40%, respectively. We observed that for every 1% increase in anthropogenic aerosols, AOD increased by 0.55% during winter whereas for every 1% increase in dust aerosols, AOD increased by 0.46% during pre-monsoon. The natural dust transport process (during pre-monsoon) plays as important a role in the radiation effects as the anthropogenic biomass burning (during winter) and their differential effects (rate of increase of the AOD with that of the aerosol concentration) are also very similar. This should be taken into account in proper modeling of the atmospheric environment over eastern Himalayas.

  8. Aerosol optical properties during firework, biomass burning and dust episodes in Beijing

    NASA Astrophysics Data System (ADS)

    Yu, Xingna; Shi, Chanzhen; Ma, Jia; Zhu, Bin; Li, Mei; Wang, Jing; Yang, Suying; Kang, Na

    2013-12-01

    In order to characterize the aerosol optical properties during different pollution episodes that occurred in Beijing, the aerosol loading, scattering, and size distributions are presented using solar and sky radiance measurements from 2001 to 2010 in this paper. A much higher aerosol loading than the background level was observed during the pollution episodes. The average aerosol optical depth (AOD) is largest during dust episodes coupled with the lowest Ångström exponent (α), while higher AOD and lower α were more correlated with firework and biomass burning days. The total mean AOD at 440, 675, 870 and 1020 nm were 0.24, 0.49, 0.64 and 1.38 in the clean, firework display, biomass burning and dust days, respectively. The mean α for dust days was 0.51 and exceeded 1.1 for the remaining episodes. The size distribution of the dusty periods was dominated by the coarse mode, but the coarse mode was similar magnitude to the fine mode during the firework and biomass burning days. The volume concentration of the coarse mode during the dust days increased by a magnitude of more than 2-8 times that derived in the other three aerosol conditions, suggesting that dust is the major contributor of coarse mode particles in Beijing. The single scattering albedo (SSA) values also increased during the pollution episodes. The overall mean SSA at the four wavelengths were 0.865, 0.911, 0.922 and 0.931 in clean, firework display, biomass burning, and dust days in Beijing, respectively. However, in the blue spectral range, the dust aerosols exhibited pronounced absorption.

  9. Improving aerosol vertical retrieval for NWP application: Studying the impact of IR-sensed aerosol on data assimilation systems.

    NASA Astrophysics Data System (ADS)

    Oyola, Mayra; Marquis, Jared; Ruston, Benjamin; Campbell, James; Baker, Nancy; Westphal, Douglas; Zhang, Jianglong; Hyer, Edward

    2017-04-01

    Radiometric measurements from passive infrared (IR) sensors are important in numerical weather prediction (NWP) because they are sensitive to surface temperatures and atmospheric temperature profiles. However, these measurements are also sensitive to absorbing and scattering constituents in the atmosphere. Dust aerosols absorb in the IR and are found over many global regions with irregular spatial and temporal frequency. Retrievals of temperature using IR data are thus vulnerable to dust-IR radiance biases, most notably over tropical oceans where accurate surface and atmospheric temperatures are critical to accurate prediction of tropical cyclone development. Previous studies have shown that dust aerosols can bias retrieved brightness temperatures (BT) by up to 10K in some IR channels that are assimilated to constrain atmospheric temperature and water vapor profiles. Other BT-derived parameters such as sea surface temperatures (SSTs) are susceptible to negative biases of at least 1K or higher, which conflicts with the accuracy requirement for most research and operational applications (i.e., +/- 0.3 K). This problem is not limited to just satellite retrievals. BT bias also impacts the incorporation of background fields from NWP analyses in data assimilation (DA) systems. The effect of aerosols on IR fluxes at the ocean surface is a function of both aerosol loading and vertical profile. Therefore, knowledge of the aerosol vertical distribution, and understanding of how well this distribution is captured by NWP models, is necessary to ensuring proper treatment of aerosol-affected radiances in both retrieval and data assimilation. This understanding can be achieved by conducting modeling studies and by the exploitation of a robust observational dataset, such as satellite-based lidar profiling, which can be used to characterize aerosol type and distribution. In this talk, we describe such an application using the Navy Aerosol Analysis Prediction System (NAAPS) and

  10. Modeling investigation of light-absorbing aerosols in the Amazon Basin during the wet season

    NASA Astrophysics Data System (ADS)

    Wang, Qiaoqiao; Saturno, Jorge; Chi, Xuguang; Walter, David; Lavric, Jost; Moran-Zuloaga, Daniel; Ditas, Florian; Pöhlker, Christopher; Brito, Joel; Carbone, Samara; Artaxo, Paulo; Andreae, Meinrat

    2017-04-01

    We use a global chemical transport model (GEOS-Chem) to interpret observed light-absorbing aerosols in Amazonia during the wet season. Observed aerosol properties, including black carbon (BC) concentration and light absorption, at the Amazon Tall Tower Observatory (ATTO) site in the central Amazon have relatively low background levels but frequently show high peaks during the study period of January-April 2014. With daily temporal resolution for open fire emissions and modified aerosol optical properties, our model successfully captures the observed variation in fine/coarse aerosol and BC concentrations as well as aerosol light absorption and its wavelength dependence over the Amazon Basin. The source attribution in the model indicates the important influence of open fire on the observed variances of aerosol concentrations and absorption, mainly from regional sources (northern South America) and from northern Africa. The contribution of open fires from these two regions is comparable, with the latter becoming more important in the late wet season. The analysis of correlation and enhancement ratios of BC versus CO suggests transport times of < 3 days for regional fires and 11 days for African plumes arriving at ATTO during the wet season. The model performance of long-range transport of African plumes is also evaluated with observations from AERONET, MODIS, and CALIOP. Simulated absorption aerosol optical depth (AAOD) averaged over the wet season is lower than 0.0015 over the central Amazon, including the ATTO site. We find that more than 50% of total absorption at 550 nm is from BC, except for the northeastern Amazon and the Guianas, where the influence of dust becomes significant (up to 35 %). The brown carbon contribution is generally between 20 and 30 %. The distribution of absorption Ångström exponents (AAE) suggests more influence from fossil fuel combustion in the southern part of the basin (AAE 1) but more open fire and dust influence in the northern part

  11. Remote sensing of aerosols by synergy of caliop and modis

    NASA Astrophysics Data System (ADS)

    Kudo, Rei; Nishizawa, Tomoaki; Higurashi, Akiko; Oikawa, Eiji

    2018-04-01

    For the monitoring of the global 3-D distribution of aerosol components, we developed the method to retrieve the vertical profiles of water-soluble, light absorbing carbonaceous, dust, and sea salt particles by the synergy of CALIOP and MODIS data. The aerosol product from the synergistic method is expected to be better than the individual products of CALIOP and MODIS. We applied the method to the biomass-burning event in Africa and the dust event in West Asia. The reasonable results were obtained; the much amount of the water-soluble and light absorbing carbonaceous particles were estimated in the biomass-burning event, and the dust particles were estimated in the dust event.

  12. New capabilities for characterizing smoke and dust aerosol over land using MODIS

    NASA Astrophysics Data System (ADS)

    Levy, R. C.; Remer, L. A.

    2006-12-01

    Smoke and dust aerosol have different chemical, optical and physical properties and both types affect many processes within the climate system. As earth's surface and atmosphere are continuously altered by natural and anthropogenic processes, the emission and presumably the effects of these aerosols are also changing. Thus it is necessary to observe and characterize aerosols on a global and climatic scale. While MODIS has been reporting characteristics of smoke and dust aerosol over land and ocean since shortly after Terra launch, the uncertainties in the over-land retrieval have been larger than expected. To better characterize different aerosol types closer to their source regions with greater accuracy, we have developed a new operational algorithm for retrieving aerosol properties over dark land surfaces from MODIS-observed visible (VIS) and infrared (IR) reflectance. Like earlier versions, this algorithm estimates the total loading (aerosol optical depth-τ) and relative weighting of fine (non-dust) and coarse (dust) -dominated aerosol to the total τ (fine weighting-η) over dark land surfaces. However, the fundamental mathematics and major assumptions have been overhauled. The new algorithm performs simultaneous multi-channel inversion that includes information about coarse aerosol in the IR channels, while assuming a fine-tuned relationship between VIS and IR surface reflectances, that is itself a function of scattering angle and vegetation condition. Finally, the suite of expected aerosol optical models described by the lookup table have been revised to closer resemble the AERONET climatology, including for smoke and dust aerosol. Beginning in April 2006, this algorithm has been used for forward processing and backward re- processing of the entire MODIS dataset observed from both Terra and Aqua. "Collection 5" products were completed for Aqua reprocessing by July 2006 and should be complete for Terra by December 2006. In this study, we used the complete

  13. Temporal and spatial characteristics of dust devils and their contribution to the aerosol budget in East Asia-An analysis using a new parameterization scheme for dust devils

    NASA Astrophysics Data System (ADS)

    Tang, Yaoguo; Han, Yongxiang; Liu, Zhaohuan

    2018-06-01

    Dust aerosols are the main aerosol components of the atmosphere that affect climate change, but the contribution of dust devils to the atmospheric dust aerosol budget is uncertain. In this study, a new parameterization scheme for dust devils was established and coupled with WRF-Chem, and the diurnal and monthly variations and the contribution of dust devils to the atmospheric dust aerosol budget in East Asia was simulated. The results show that 1) both the diurnal and monthly variations in dust devil emissions in East Asia had unimodal distributions, with peaks in the afternoon and the summer that were similar to the observations; 2) the simulated dust devils occurred frequently in deserts, including the Gobi. The distributed area and the intensity center of the dust devil moved from east to west during the day; 3) the ratio between the availability of convective buoyancy relative to the frictional dissipation was the main factor that limited the presence of dust devils. The position of the dust devil formation, the surface temperature, and the boundary layer height determined the dust devil intensity; 4) the contribution of dust devils to atmospheric dust aerosols determined in East Asia was 30.4 ± 13%, thereby suggesting that dust devils contribute significantly to the total amount of atmospheric dust aerosols. Although the new parameterization scheme for dust devils was rough, it was helpful for understanding the distribution of dust devils and their contribution to the dust aerosol budget.

  14. Numerical simulations of Asian dust storms using a coupled climate-aerosol microphysical model

    NASA Astrophysics Data System (ADS)

    Su, Lin; Toon, Owen B.

    2009-07-01

    We have developed a three-dimensional coupled microphysical/climate model based on the National Center for Atmospheric Research Community Atmospheres Model and the University of Colorado/NASA Community Aerosol and Radiation Model for Atmospheres. We have used the model to investigate the sources, removal processes, transport, and optical properties of Asian dust aerosol and its impact on downwind regions. The model simulations are conducted primarily during the time frame of the Aerosol Characterization Experiment-Asia field experiment (March-May 2001) since considerable in situ data are available at that time. Our dust source function follows Ginoux et al. (2001). We modified the dust source function by using the friction velocity instead of the 10-m wind based on wind erosion theory, by adding a size-dependent threshold friction velocity following Marticorena and Bergametti (1995) and by adding a soil moisture correction. A Weibull distribution is implemented to estimate the subgrid-scale wind speed variability. We use eight size bins for mineral dust ranging from 0.1 to 10 μm radius. Generally, the model reproduced the aerosol optical depth retrieved by the ground-based Aerosol Robotic Network (AERONET) Sun photometers at six study sites ranging in location from near the Asian dust sources to the Eastern Pacific region. By constraining the dust complex refractive index from AERONET retrievals near the dust source, we also find the single-scattering albedo to be consistent with AERONET retrievals. However, large regional variations are observed due to local pollution. The timing of dust events is comparable to the National Institute for Environmental Studies (NIES) lidar data in Beijing and Nagasaki. However, the simulated dust aerosols are at higher altitudes than those observed by the NIES lidar.

  15. Observed high aerosol loading during dust events in Delhi

    NASA Astrophysics Data System (ADS)

    Singh, Khem; Aggarwal, Shankar G.; Jha, Arvind K.; Singh, Nahar; Soni, Daya; Gupta, Prabhat K.

    2012-07-01

    The present study reports aerosol mass loadings and their chemical property during integrated campaign for aerosol and radiation budget (ICARB) in the month of March to May 2006, at NPL, New Delhi. The Thar Desert in Rajasthan is located on the western end of India and south-west of Delhi is hot and arid region with intense aeolian activity and transport of aerosol by the prevailing southwest-west summer wind. Several dust episodes were observed in Delhi during summer 2006. The dust storm peaked on 29th April, 1 ^{st} and 8 ^{th} May 2006, with very high suspended particulate matter (SPM) concentrations 1986μg/m ^{3}, 1735μg/m ^{3} and 1511μg/m ^{3}, respectively. The average concentration of SPM in the month of March, April and May 2006 was 338 μg/m ^{3}, 698 μg/m ^{3} and 732 μg/m ^{3}, respectively. The SPM filter samples were analysed for water-soluble major cations (Na ^{+}, Ca ^{2+}, K ^{+}, and Mg ^{2+}) by atomic absorption spectrophotometry (AAS). Na ^{+} and Ca ^{2+} contribute about 54% and 20%, respectively of the total identified cation mass, indicating that they were most abundant cations. Strong correlations between Na ^{+}, Ca ^{2+}, K ^{+}, and Mg ^{2+} suggest their soil and dust origin. Such a high particle concentration observed during dust events may also be useful for study the effect of these aerosols on communication medium.

  16. Regional transport of anthropogenic pollution and dust aerosols in spring to Tianjin - A coastal megacity in China.

    PubMed

    Su, Xiaoli; Wang, Qiao; Li, Zhengqiang; Calvello, Mariarosaria; Esposito, Francesco; Pavese, Giulia; Lin, Meijing; Cao, Junji; Zhou, Chunyan; Li, Donghui; Xu, Hua

    2017-04-15

    Simultaneous measurements of columnar aerosol microphysical and optical properties, as well as PM 2.5 chemical compositions, were made during two types of spring pollution episodes in Tianjin, a coastal megacity of China. The events were investigated using field observations, satellite data, model simulations, and meteorological fields. The lower Ångström Exponent and the higher aerosol optical depth on 29 March, compared with the earlier event on 26 March, implied a dominance of coarse mode particles - this was consistent with the differences in volume-size distributions. Based on the single scattering spectra, the dominant absorber (at blue wavelength) changed from black carbon during less polluted days to brown carbon on 26 March and dust on 29 March. The concentrations of major PM 2.5 species for these two episodes also differed, with the earlier event enriched in pollution-derived substances and the later with mineral dust elements. The formation mechanisms of these two pollution episodes were also examined. The 26 March episode was attributed to the accumulation of both local emissions and anthropogenic pollutants transported from the southwest of Tianjin under the control of high pressure system. While the high aerosol loading on 29 March was caused by the mixing of transported dust from northwest source region with local urban pollution. The mixing of transported anthropogenic pollutants and dust with local emissions demonstrated the complexity of springtime pollution in Tianjin. The synergy of multi-scale observations showed excellent potential for air pollution study. Copyright © 2017 Elsevier B.V. All rights reserved.

  17. Examination of the potential impacts of dust and pollution aerosol acting as cloud nucleating aerosol on water resources in the Colorado River Basin

    NASA Astrophysics Data System (ADS)

    Jha, Vandana

    In this study we examine the cumulative effect of dust acting as cloud nucleating aerosol (cloud condensation nuclei (CCN), giant cloud condensation nuclei (GCCN), and ice nuclei (IN)) along with anthropogenic aerosol pollution acting primarily as CCN, over the entire Colorado Rocky Mountains from the months of October to April in the year 2004-2005; the snow year. This ˜6.5 months analysis provides a range of snowfall totals and variability in dust and anthropogenic aerosol pollution. The specific objectives of this research is to quantify the impacts of both dust and pollution aerosols on wintertime precipitation in the Colorado Mountains using the Regional Atmospheric Modeling System (RAMS). In general, dust enhances precipitation primarily by acting as IN, while aerosol pollution reduces water resources in the CRB via the so-called "spill-over" effect, by enhancing cloud droplet concentrations and reducing riming rates. Dust is more episodic and aerosol pollution is more pervasive throughout the winter season. Combined response to dust and aerosol pollution is a net reduction of water resources in the CRB. The question is by how much are those water resources affected? Our best estimate is that total winter-season precipitation loss for for the CRB the 2004-2005 winter season due to the combined influence of aerosol pollution and dust is 5,380,00 acre-feet of water. Sensitivity studies for different cases have also been run for the specific cases in 2004-2005 winter season to analyze the impact of changing dust and aerosol ratios on precipitation in the Colorado River Basin. The dust is varied from 3 to 10 times in the experiments and the response is found to be non monotonic and depends on various environmental factors. The sensitivity studies show that adding dust in a wet system increases precipitation when IN affects are dominant. For a relatively dry system high concentrations of dust can result in over-seeding the clouds and reductions in precipitation

  18. Radiative forcing by light-absorbing aerosols of pyrogenetic iron oxides.

    PubMed

    Ito, Akinori; Lin, Guangxing; Penner, Joyce E

    2018-05-09

    Iron (Fe) oxides in aerosols are known to absorb sun light and heat the atmosphere. However, the radiative forcing (RF) of light-absorbing aerosols of pyrogenetic Fe oxides is ignored in climate models. For the first time, we use a global chemical transport model and a radiative transfer model to estimate the RF by light-absorbing aerosols of pyrogenetic Fe oxides. The model results suggest that strongly absorbing Fe oxides (magnetite) contribute a RF that is about 10% of the RF due to black carbon (BC) over East Asia. The seasonal average of the RF due to dark Fe-rich mineral particles over East Asia (0.4-1.0 W m -2 ) is comparable to that over major biomass burning regions. This additional warming effect is amplified over polluted regions where the iron and steel industries have been recently developed. These findings may have important implications for the projection of the climate change, due to the rapid growth in energy consumption of the heavy industry in newly developing countries.

  19. Systematic Relationships Between Lidar Observables and Sizes And Mineral Composition Of Dust Aerosols

    NASA Technical Reports Server (NTRS)

    Van Diedenhoven, Bastiaan; Stangl, Alexander; Perlwitz, Jan; Fridlind, Ann M.; Chowdhary, Jacek; Cairns, Brian

    2015-01-01

    The physical and chemical properties of soil dust aerosol particles fundamentally affect their interaction with climate, including shortwave absorption and radiative forcing, nucleation of cloud droplets and ice crystals, heterogeneous formation of sulfates and nitrates on the surface of dust particles, and atmospheric processing of iron into bioavailable forms that increase the productivity of marine phytoplankton. Lidar measurements, such as extinction-to-backscatter, color and depolarization ratios, are frequently used to distinguish between aerosol types with different physical and chemical properties. The chemical composition of aerosol particles determines their complex refractive index, hence affecting their backscattering properties. Here we present a study on how dust aerosol backscattering and depolarization properties at wavelengths of 355, 532 and 1064 nm are related to size and complex refractive index, which varies with the mineral composition of the dust. Dust aerosols are represented by collections of spheroids with a range of prolate and oblate aspect ratios and their optical properties are obtained using T-matrix calculations. We find simple, systematic relationships between lidar observables and the dust size and complex refractive index that may aid the use of space-based or airborne lidars for direct retrieval of dust properties or for the evaluation of chemical transport models using forward simulated lidar variables. In addition, we present first results on the spatial variation of forward-simulated lidar variables based on a dust model that accounts for the atmospheric cycle of eight different mineral types plus internal mixtures of seven mineral types with iron oxides, which was recently implemented in the NASA GISS Earth System ModelE2.

  20. Dust aerosol radiative effect and influence on urban atmospheric boundary layer

    NASA Astrophysics Data System (ADS)

    Zhang, L.; Chen, M.; Li, L.

    2007-11-01

    An 1.5-level-closure and 3-D non-stationary atmospheric boundary layer (ABL) model and a radiation transfer model with the output of Weather Research and Forecast (WRF) Model and lidar AML-1 are employed to simulate the dust aerosol radiative effect and its influence on ABL in Beijing for the period of 23-26 January 2002 when a dust storm occurred. The simulation shows that daytime dust aerosol radiative effect heats up the ABL at the mean rate of about 0.68 K/h. The horizontal wind speed from ground to 900 m layer is also overall increased, and the value changes about 0.01 m/s at 14:00 LT near the ground. At night, the dust aerosol radiative effect cools the ABL at the mean rate of -0.21 K/h and the wind speed lowers down at about -0.19 m/s at 02:00 LT near the ground.

  1. Cloud Cover Increase with Increasing Aerosol Absorptivity: A Counterexample to the Conventional Semidirect Aerosol Effect

    NASA Technical Reports Server (NTRS)

    Perlwitz, Jan; Miller, Ron L.

    2010-01-01

    We reexamine the aerosol semidirect effect using a general circulation model and four cases of the single-scattering albedo of dust aerosols. Contrary to the expected decrease in low cloud cover due to heating by tropospheric aerosols, we find a significant increase with increasing absorptivity of soil dust particles in regions with high dust load, except during Northern Hemisphere winter. The strongest sensitivity of cloud cover to dust absorption is found over land during Northern Hemisphere summer. Here even medium and high cloud cover increase where the dust load is highest. The cloud cover change is directly linked to the change in relative humidity in the troposphere as a result of contrasting changes in specific humidity and temperature. More absorption by aerosols leads to larger diabatic heating and increased warming of the column, decreasing relative humidity. However, a corresponding increase in the specific humidity exceeds the temperature effect on relative humidity. The net effect is more low cloud cover with increasing aerosol absorption. The higher specific humidity where cloud cover strongly increases is attributed to an enhanced convergence of moisture driven by dust radiative heating. Although in some areas our model exhibits a reduction of low cloud cover due to aerosol heating consistent with the conventional description of the semidirect effect, we conclude that the link between aerosols and clouds is more varied, depending also on changes in the atmospheric circulation and the specific humidity induced by the aerosols. Other absorbing aerosols such as black carbon are expected to have a similar effect.

  2. Remote Sensing of Aerosol and Non-Aerosol Absorption

    NASA Technical Reports Server (NTRS)

    Kaufman, Y. J.; Dubovik, O.; Holben, B. N.; Remer, L. A.; Tanre, D.; Lau, William K. M. (Technical Monitor)

    2001-01-01

    Remote sensing of aerosol from the new satellite instruments (e.g. MODIS from Terra) and ground based radiometers (e.g. the AERONET) provides the opportunity to measure the absorption characteristics of the ambient undisturbed aerosol in the entire atmospheric column. For example Landsat and AERONET data are used to measure spectral absorption of sunlight by dust from West Africa. Both Application of the Landsat and AERONET data demonstrate that Saharan dust absorption of solar radiation is several times smaller than the current international standards. This is due to difficulties of measuring dust absorption in situ, and due to the often contamination of dust properties by the presence of air pollution or smoke. We use the remotely sensed aerosol absorption properties described by the spectral sin le scattering albedo, together with statistics of the monthly optical thickness for the fine and coarse aerosol derived from the MODIS data. The result is an estimate of the flux of solar radiation absorbed by the aerosol layer in different regions around the globe where aerosol is prevalent. If this aerosol forcing through absorption is not included in global circulation models, it may be interpreted as anomalous absorption in these regions. In a preliminary exercise we also use the absorption measurements by AERONET, to derive the non-aerosol absorption of the atmosphere in cloud free conditions. The results are obtained for the atmospheric windows: 0.44 microns, 0.66 microns, 0.86 microns and 1.05 microns. In all the locations over the land and ocean that were tested no anomalous absorption in these wavelengths, was found within absorption optical thickness of +/- 0.005.

  3. Satellite remote sensing of dust aerosol indirect effects on ice cloud formation.

    PubMed

    Ou, Steve Szu-Cheng; Liou, Kuo-Nan; Wang, Xingjuan; Hansell, Richard; Lefevre, Randy; Cocks, Stephen

    2009-01-20

    We undertook a new approach to investigate the aerosol indirect effect of the first kind on ice cloud formation by using available data products from the Moderate-Resolution Imaging Spectrometer (MODIS) and obtained physical understanding about the interaction between aerosols and ice clouds. Our analysis focused on the examination of the variability in the correlation between ice cloud parameters (optical depth, effective particle size, cloud water path, and cloud particle number concentration) and aerosol optical depth and number concentration that were inferred from available satellite cloud and aerosol data products. Correlation results for a number of selected scenes containing dust and ice clouds are presented, and dust aerosol indirect effects on ice clouds are directly demonstrated from satellite observations.

  4. Does variation in mineral composition alter the short-wave light scattering properties of desert dust aerosol?

    NASA Astrophysics Data System (ADS)

    Smith, Andrew J. A.; Grainger, Roy G.

    2014-01-01

    Mineral dust aerosol is a major component of natural airborne particulates. Using satellite measurements from the visible and near-infrared, there is insufficient information to retrieve a full microphysical and chemical description of an aerosol distribution. As such, refractive index is one of many parameters that must be implicitly assumed in order to obtain an optical depth retrieval. This is essentially a proxy for the dust mineralogy. Using a global soil map, it is shown that as long as a reasonable refractive index for dust is assumed, global dust variability is unlikely to cause significant variation in the optical properties of a dust aerosol distribution in the short-wave, and so should not greatly affect retrievals of mineral dust aerosol from space by visible and near-infrared radiometers. Errors in aerosol optical depth due to this variation are expected to be ≲ 1 %. The work is framed around the ORAC AATSR aerosol retrieval, but is equally applicable to similar satellite retrievals. In this case, variations in the top-of-atmosphere reflectance caused by mineral variation are within the noise limits of the instrument.

  5. Analysis of the Impact of Major Dust Events on the Aerosols Characteristics over Saudi Arabia

    NASA Astrophysics Data System (ADS)

    Farahat, Ashraf; El-Askary, Hesham; Al-Shaibani, Abdulaziz; Hariri, Mustafa M.

    2015-04-01

    The Kingdom of Saudi Arabia is a major source of atmospheric dust. Frequent dust storms blow up and significantly affect human activities, airports and citizens' health. Aerosols optical and physical characteristics are influenced by major dust storms outbreaks. In this, paper, ground based AERONET measurements are integrated with space-borne sensors, namely MODIS and CALIPSO to analyze aerosols' characteristics during March - May of 2009 where a massive dust storm blew up and caused a widespread heavy atmospheric dust load over Saudi Arabia and the same period during 2010, where less dust activities were reported. The MODIS Deep Blue AOD analysis showed similar aerosols pattern over the land, however a substantial variance in aerosol loading during March - May 2009 compared with the same period in 2010 was observed. The angstrom exponent analysis showed that the majority of aerosol measurements in 2009 and 2010 are dominated by coarse-mode particles with angstrom exponent < 0.5. Detailed analysis of aerosol optical properties shows significant influence of coarse mode particles in the enhanced aerosol loading in 2009. The volume depolarization rations (VDR) derived from CALIPSO backscattering measurements is used to find latitudinal profile of mean aerosol optical depth to indicate the type of particles and to discriminate spherical aerosols with non-spherical particles. Acknowledgement The authors would like to acknowledge the support provided by the King Abdel Aziz City for Science & Technology (KACST) for funding this work under grant No. (MT-32-76). The support provided by the Deanship of Research at King Fahd University of Petroleum & Minerals (KFUPM) is gratefully acknowledged.

  6. Long term change in atmospheric dust absorption, dust scattering and black carbon aerosols scattering coefficient parameters over western Indian locations

    NASA Astrophysics Data System (ADS)

    Satoliya, Anil Kumar; Vyas, B. M.; Shekhawat, M. S.

    2018-05-01

    The first time satellite space based measurement of atmospheric black carbon (BC) aerosols scattering coefficient at 550nm (BC SC at 550nm), dust aerosols scattering and dust aerosols extinction coefficient (DSC at 550nm and DEC at 550nm) parameters have been used to understand their long term trend of natural and anthropogenic aerosols behavior with its close association with ground based measured precipitation parameters such as Total Rain Fall (TRF), and Total Number of Rainy Days (TNRD) for the same period over western Indian regions concerned to the primary aerosols sources of natural activities. The basic objective of this study is an attempt to investigate the inter-correlation between dust and black carbon aerosols loading characteristics with a variation of rainfall pattern parameters as indirect aerosols induced effect i.e., aerosols-cloud interaction. The black carbon aerosols generated by diverse anthropogenic or human made activities are studied by choosing of measured atmospheric BC SC at 550nm parameter, whereas desert dust mineral aerosols primarily produced by varieties of natural activities pre-dominated of dust mineral desert aerosols mainly over Thar desert influenced area of hot climate and rural tropical site are investigated by selecting DSC at 550nm and DEC at 550nm of first semi-urban site i.e., Udaipur (UDP, 24.6°N, 73.35°E, 580m above surface level (asl)) situated in southern Rajasthan part as well as over other two Great Indian Thar desert locations i.e., Jaisalmer (JSM, 26.90°N, 69.90°E, 220m asl)) and Bikaner (BKN, 28.03°N, 73.30°E, 224m asl) located in the vicinity of the Thar desert region situated in Rajasthan state of the western Indian region. The source of the present study would be collection of longer period of monthly values of the above parameters of spanning 35 years i.e., 1980 to 2015. Such types of atmospheric aerosols-cloud monsoon interaction investigation is helpful in view of understanding their direct and

  7. Distribution and radiative forcing of Asian dust and anthropogenic aerosols from East Asia simulated by SPRINTARS

    NASA Astrophysics Data System (ADS)

    Takemura, T.; Nakajima, T.; Uno, I.

    2002-12-01

    A three-dimensional aerosol transport-radiation model, SPRINTARS (Spectral Radiation-Transport Model for Aerosol Species), has been developed based on an atmospheric general circulation model of the Center for Climate System Research, University of Tokyo/National Institute for Environmental Studies, Japan to research the effects of aerosols on the climate system and atmospheric environment. SPRINTARS successfully simulates the long-range transport of the large-scale Asian dust storms from East Asia to North America by crossing the North Pacific Ocean in springtime 2001 and 2002. It is found from the calculated dust optical thickness that 10 to 20% of Asian dust around Japan reached North America. The simulation also reveals the importance of anthropogenic aerosols, which are carbonaceous and sulfate aerosols emitted from the industrialized areas in the East Asian continent, to air turbidity during the large-scale Asian dust storms. The simulated results are compared with a volume of observation data regarding the aerosol characteristics over East Asia in the spring of 2001 acquired by the intensive observation campaigns of ACE-Asia (Asian Pacific Regional Aerosol Characterization Experiment) and APEX (Asian Atmospheric Particulate Environmental Change Studies). The comparisons are carried out not only for aerosol concentrations but also for aerosol optical properties, such as optical thickness, Angstrom exponent which is a size index calculated by the log-slope exponent of the optical thickness between two wavelengths, and single scattering albedo. The consistence of Angstrom exponent between the simulation and observations means the reasonable simulation of the ratio of anthropogenic aerosols to Asian dust, which supports the suggestion by the simulation on the importance of anthropogenic aerosols to air turbidity during the large-scale Asian dust storms. SPRINTARS simultaneously calculates the aerosol direct and indirect radiative forcings. The direct radiative

  8. Vertical Distribution of Dust and Water Ice Aerosols from CRISM Limb-geometry Observations

    NASA Technical Reports Server (NTRS)

    Smith, Michael Doyle; Wolff, Michael J.; Clancy, Todd; Kleinbohl, Armin; Murchie, Scott L.

    2013-01-01

    [1] Near-infrared spectra taken in a limb-viewing geometry by the Compact Reconnaissance Imaging Spectrometer for Mars (CRISM) on board the Mars Reconnaissance Orbiter provide a useful tool for probing atmospheric structure. Specifically, the observed radiance as a function of wavelength and height above the limb enables the vertical distribution of both dust and water ice aerosols to be retrieved. More than a dozen sets of CRISM limb observations have been taken so far providing pole-to-pole cross sections, spanning more than a full Martian year. Radiative transfer modeling is used to model the observations taking into account multiple scattering from aerosols and the spherical geometry of the limb observations. Both dust and water ice vertical profiles often show a significant vertical structure for nearly all seasons and latitudes that is not consistent with the well-mixed or Conrath-v assumptions that have often been used in the past for describing aerosol vertical profiles for retrieval and modeling purposes. Significant variations are seen in the retrieved vertical profiles of dust and water ice aerosol as a function of season. Dust typically extends to higher altitudes (approx. 40-50km) during the perihelion season than during the aphelion season (<20km), and the Hellas region consistently shows more dust mixed to higher altitudes than other locations. Detached water ice clouds are common, and water ice aerosols are observed to cap the dust layer in all seasons.

  9. Dust Aerosols at the Source Region During ACE-ASIA: A Surface/Satellite Perspective

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Lau, William K. M. (Technical Monitor)

    2001-01-01

    ACE (Aerosol Characterization Experiment)-Asia is designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern Asia and along the rim of the western Pacific. The phase-I of ACE-Asia was conducted from March-May 2001 in the vicinity of the Gobi desert, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian dust is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of dust aerosol radiative flux in addition to measurements of loading and optical thickness. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. Preliminary results will be presented and discussed their implications in regional climatic effects.

  10. Assessment of dust aerosol effect on cloud properties over Northwest China using CERES SSF data

    NASA Astrophysics Data System (ADS)

    Huang, J.; Wang, X.; Wang, T.; Su, J.; Minnis, P.; Lin, B.; Hu, Y.; Yi, Y.

    Dust aerosols not only have direct effects on the climate through reflection and absorption of the short and long wave radiation but also modify cloud properties such as the number concentration and size of cloud droplets indirect effect and contribute to diabatic heating in the atmosphere that often enhances cloud evaporation and reduces the cloud water path In this study indirect and semi-direct effects of dust aerosols are analyzed over eastern Asia using two years June 2002 to June 2004 of CERES Clouds and the Earth s Radiant Energy Budget Scanner and MODIS MODerate Resolution Imaging Spectroradiometer Aqua Edition 1B SSF Single Scanner Footprint data sets The statistical analysis shows evidence for both indirect and semi-direct effect of Asia dust aerosols The dust appears to reduce the ice cloud effective particle diameter and increase high cloud amount On average ice cloud effective particle diameters of cirrus clouds under dust polluted conditions dusty cloud are 11 smaller than those derived from ice clouds in dust-free atmospheric environments The water paths of dusty clouds are also considerably smaller than those of dust-free clouds Dust aerosols could warm clouds thereby increasing the evaporation of cloud droplets resulting in reduced cloud water path semi-direct effect The semi-direct effect may be dominated the interaction between dust aerosols and clouds over arid and semi-arid areas and partly contribute to reduced precipitation

  11. Validation of MODIS Dust Aerosol Retrieval and Development Ambient Dust Phase Function using PRIDE Data

    NASA Technical Reports Server (NTRS)

    Remer, Lorraine A.; Lau, William (Technical Monitor)

    2002-01-01

    The PRIDE data set of MODIS aerosol retrievals co-located with sunphotometer measurements provides the basis of MODIS validation in a dust environment. The sunphotometer measurements include AERONET automatic instruments, land-based Microtops instruments, ship-board Microtops instruments and the AATS-6 aboard the Navajo aircraft. Analysis of these data indicate that the MODIS retrieval is within pre-launch estimates of uncertainty within the spectral range of 600-900 nm. However, the MODIS algorithm consistently retrieves smaller particles than reality thus leading to incorrect spectral response outside of the 600-900 nm range and improper size information. Further analysis of MODIS retrievals in other dust environments shows the inconsistencies are due to nonspherical effects in the phase function. These data are used to develop an ambient phase function for dust aerosol to be used for remote sensing purposes.

  12. Effects of morphology on the radiative properties of internally mixed light absorbing carbon aerosols with different aging status.

    PubMed

    Cheng, Tianhai; Wu, Yu; Chen, Hao

    2014-06-30

    Light absorbing carbon aerosols play a substantial role in climate change through radiative forcing, which is the dominant absorber of solar radiation. Radiative properties of light absorbing carbon aerosols are strongly dependent on the morphological factors and the mixing mechanism of black carbon with other aerosol components. This study focuses on the morphological effects on the optical properties of internally mixed light absorbing carbon aerosols using the numerically exact superposition T-matrix method. Three types aerosols with different aging status such as freshly emitted BC particles, thinly coated light absorbing carbon aerosols, heavily coated light absorbing carbon aerosols are studied. Our study showed that morphological factors change with the aging of internally mixed light absorbing carbon aerosols to result in a dramatic change in their optical properties. The absorption properties of light absorbing carbon aerosols can be enhanced approximately a factor of 2 at 0.67 um, and these enhancements depend on the morphological factors. A larger shell/core diameter ratio of volume-equivalent shell-core spheres (S/C), which indicates the degree of coating, leads to stronger absorption. The enhancement of absorption properties accompanies a greater enhancement of scattering properties, which is reflected in an increase in single scattering albedo (SSA). The enhancement of single scattering albedo due to the morphological effects can reach a factor of 3.75 at 0.67 μm. The asymmetry parameter has a similar yet smaller enhancement. Moreover, the corresponding optical properties of shell-and-core model determined by using Lorenz -Mie solutions are presented for comparison. We found that the optical properties of internally mixed light absorbing carbon aerosol can differ fundamentally from those calculated for the Mie theory shell-and-core model, particularly for thinly coated light absorbing carbon aerosols. Our studies indicate that the complex morphology

  13. Properties of transported African mineral dust aerosols in the Mediterranean region

    NASA Astrophysics Data System (ADS)

    Denjean, Cyrielle; Chevaillier, Servanne; Gaimoz, Cécile; Grand, Noel; Triquet, Sylvain; Zapf, Pascal; Loisil, Rodrigue; Bourrianne, Thierry; Freney, Evelyn; Dupuy, Regis; Sellegri, Karine; Schwarzenbock, Alfons; Torres, Benjamin; Mallet, Marc; Cassola, Federico; Prati, Paolo; Formenti, Paola

    2015-04-01

    The transport of mineral dust aerosols is a global phenomenon with strong climate implications. Depending on the travel distance over source regions, the atmospheric conditions and the residence time in the atmosphere, various transformation processes (size-selective sedimentation, mixing, condensation of gaseous species, and weathering) can modify the physical and chemical properties of mineral dust, which, in turn, can change the dust's optical properties. The model predictions of the radiative effect by mineral dust still suffer of the lack of certainty of these properties, and their temporal evolution with transport time. Within the frame of the ChArMex project (Chemistry-Aerosol Mediterranean experiment, http://charmex.lsce.ipsl.fr/), one intensive airborne campaign (ADRIMED, Aerosol Direct Radiative Impact in the regional climate in the MEDiterranean region, 06 June - 08 July 2013) has been performed over the Central and Western Mediterranean, one of the two major transport pathways of African mineral dust. In this study we have set up a systematic strategy to determine the optical, physical and optical properties of mineral dust to be compared to an equivalent dataset for dust close to source regions in Africa. This study is based on airborne observations onboard the SAFIRE ATR-42 aircraft, equipped with state of the art in situ instrumentation to measure the particle scattering and backscattering coefficients (nephelometer at 450, 550, and 700 nm), the absorption coefficient (PSAP at 467, 530, and 660 nm), the extinction coefficient (CAPS at 530 nm), the aerosol optical depth (PLASMA at 340 to 1640 nm), the size distribution in the extended range 40 nm - 30 µm by the combination of different particle counters (SMPS, USHAS, FSSP, GRIMM) and the chemical composition obtained by filter sampling. The chemistry and transport model CHIMERE-Dust have been used to classify the air masses according to the dust origin and transport. Case studies of dust transport

  14. Aerosol absorption measurements and retrievals in shadow2 campaign

    NASA Astrophysics Data System (ADS)

    Hu, Qiaoyun; Goloub, Philippe; Podvin, Thierry; Veselovskiy, Igor; Lopatin, Anton; Dubovik, Oleg; Torres, Benjamìn; Revilini, Laura; Crumeyrolle, Suzanne; Lapionak, Tatsiana; Deroo, Christine

    2018-04-01

    Dust, maritime and dust-smoke mixture events observed during SHADOW2 (SaHAran Dust Over West Africa) field campaign are selected and analyzed by using Raman and GARRLiC retrievals. The derived aerosol optical and microphysical properties will be shown. Dust absorption profile and on ground level are derived from GARRLiC retrievals and Aethalometer measurements, respectively. Our results provide a closer insight about dust absorbing properties.

  15. Observational Constraints on Ephemeral Wind Gusts that MobilizeSoil Dust Aerosols

    NASA Astrophysics Data System (ADS)

    Miller, R. L.; Leung, M. F.

    2017-12-01

    Dust aerosol models resolve the planetary scale winds that disperse particles throughout the globe, but the winds raising dust are often organized on smaller scales that are below the resolution of the model. These winds, including ephemeral wind gusts associated with boundary layer mixing, are typically parameterized. For example, gusts by dry convective eddies are related to the sensible heat flux. What remains is to constrain the magnitude of the wind gusts using boundary layer measurements, so that dust emission has the correct sensitivity to these gusts, relative to the resolved wind. Here, we use a year of ARM measurements with high temporal resolution from Niamey, Niger in the Sahel to evaluate our parameterization. This evaluation is important for dust aerosol models that use 'nudging' to reproduce observed transport patterns.

  16. Dust-wind interactions can intensify aerosol pollution over eastern China.

    PubMed

    Yang, Yang; Russell, Lynn M; Lou, Sijia; Liao, Hong; Guo, Jianping; Liu, Ying; Singh, Balwinder; Ghan, Steven J

    2017-05-11

    Eastern China has experienced severe and persistent winter haze episodes in recent years due to intensification of aerosol pollution. In addition to anthropogenic emissions, the winter aerosol pollution over eastern China is associated with unusual meteorological conditions, including weaker wind speeds. Here we show, based on model simulations, that during years with decreased wind speed, large decreases in dust emissions (29%) moderate the wintertime land-sea surface air temperature difference and further decrease winds by -0.06 (±0.05) m s -1 averaged over eastern China. The dust-induced lower winds enhance stagnation of air and account for about 13% of increasing aerosol concentrations over eastern China. Although recent increases in anthropogenic emissions are the main factor causing haze over eastern China, we conclude that natural emissions also exert a significant influence on the increases in wintertime aerosol concentrations, with important implications that need to be taken into account by air quality studies.

  17. Dust-wind interactions can intensify aerosol pollution over eastern China

    PubMed Central

    Yang, Yang; Russell, Lynn M.; Lou, Sijia; Liao, Hong; Guo, Jianping; Liu, Ying; Singh, Balwinder; Ghan, Steven J.

    2017-01-01

    Eastern China has experienced severe and persistent winter haze episodes in recent years due to intensification of aerosol pollution. In addition to anthropogenic emissions, the winter aerosol pollution over eastern China is associated with unusual meteorological conditions, including weaker wind speeds. Here we show, based on model simulations, that during years with decreased wind speed, large decreases in dust emissions (29%) moderate the wintertime land–sea surface air temperature difference and further decrease winds by −0.06 (±0.05) m s−1 averaged over eastern China. The dust-induced lower winds enhance stagnation of air and account for about 13% of increasing aerosol concentrations over eastern China. Although recent increases in anthropogenic emissions are the main factor causing haze over eastern China, we conclude that natural emissions also exert a significant influence on the increases in wintertime aerosol concentrations, with important implications that need to be taken into account by air quality studies. PMID:28492276

  18. Competing Atmospheric and Surface-Driven Impacts of Absorbing Aerosols on the East Asian Summer Monsoon

    NASA Astrophysics Data System (ADS)

    Persad, G.; Paynter, D.; Ming, Y.; Ramaswamy, V.

    2015-12-01

    Absorbing aerosols, by attenuating shortwave radiation within the atmosphere and reemitting it as longwave radiation, redistribute energy both vertically within the surface-atmosphere column and horizontally between polluted and unpolluted regions. East Asia has the largest concentrations of anthropogenic absorbing aerosols globally, and these, along with the region's scattering aerosols, have both reduced the amount of solar radiation reaching the Earth's surface regionally ("solar dimming") and increased shortwave absorption within the atmosphere, particularly during the peak months of the East Asian Summer Monsoon (EASM). We here analyze how atmospheric absorption and surface solar dimming compete in driving the response of EASM circulation to anthropogenic absorbing aerosols, which dominates, and why—issues of particular importance for predicting how the EASM will respond to projected changes in absorbing and scattering aerosol emissions in the future. We probe these questions in a state-of-the-art general circulation model (GCM) using a combination of realistic and idealized aerosol perturbations that allow us to analyze the relative influence of absorbing aerosols' atmospheric and surface-driven impacts on EASM circulation. In combination, our results make clear that, although absorption-driven dimming has a less detrimental effect on EASM circulation than purely scattering-driven dimming, aerosol absorption is still a net impairment to EASM strength when both its atmospheric and surface effects are considered. Because atmospheric heating is not efficiently conveyed to the surface, the surface dimming and associated cooling from even a pure absorber is sufficient to counteract its atmospheric heating, resulting in a net reduction in EASM strength. These findings elevate the current understanding of the impacts of aerosol absorption on the EASM, improving our ability to diagnose EASM responses to current and future regional changes in aerosol emissions.

  19. Evaluation on Asian Dust Aerosol and Simulated Processes in CanAM4.2 Using Satellite Measurements and Station Data

    NASA Astrophysics Data System (ADS)

    Yiran, P.; Li, J.; von Salzen, K.; Dai, T.; Liu, D.

    2014-12-01

    Mineral dust is a significant contributor to global and Asian aerosol burden. Currently, large uncertainties still exist in simulated aerosol processes in global climate models (GCMs), which lead to a diversity in dust mass loading and spatial distribution of GCM projections. In this study, satellite measurements from CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) and observed aerosol data from Asian stations are compared with modelled aerosol in the Canadian Atmospheric Global Climate Model (CanAM4.2). Both seasonal and annual variations in Asian dust distribution are investigated. Vertical profile of simulated aerosol in troposphere is evaluated with CALIOP Level 3 products and local observed extinction for dust and total aerosols. Physical processes in GCM such as horizontal advection, vertical mixing, dry and wet removals are analyzed according to model simulation and available measurements of aerosol. This work aims to improve current understanding of Asian dust transport and vertical exchange on a large scale, which may help to increase the accuracy of GCM simulation on aerosols.

  20. Aerosol optical, microphysical and radiative forcing properties during variable intensity African dust events in the Iberian Peninsula

    NASA Astrophysics Data System (ADS)

    Fernández, A. J.; Molero, F.; Salvador, P.; Revuelta, A.; Becerril-Valle, M.; Gómez-Moreno, F. J.; Artíñano, B.; Pujadas, M.

    2017-11-01

    Aerosol measurements at two AERONET (AErosol RObotic NETwork) sites of the Iberian Peninsula: Madrid (40°.45N, 3.72W) and La Coruña (43°.36N, 8°.42W) have been analyzed for the period 2012-2015 to assess aerosol optical properties (intensive and extensive) throughout the atmospheric column and their radiative forcing (RF) and radiative forcing efficiency (RFeff) estimates at the Bottom and Top Of Atmosphere (BOA and TOA respectively). Specific conditions as dust-free and African dust have been considered for the study. Unprecedented, this work uses the quantification of the African dust aerosol at ground level which allows us to study such AERONET products at different intensity levels of African events: Low (L), High (H) and very high (VH). The statistical difference between dust-free and African dust conditions on the aforementioned parameters, quantified by means of the non-parametric Kolmogorov-Smirnov test, is quite clear in Madrid, however it is not in La Coruña. Scattering Angstrom Exponent (SAE) and Absorption Angstrom Exponent (AAE) were found to be 1.64 ± 0.29 and 1.14 ± 0.23 respectively in Madrid for dust-free conditions because typical aerosol sources are traffic emissions and residential heating, and black carbon is an important compound in this aerosol kind. On the other hand, SAE and AAE were 0.96 ± 0.60 and 1.44 ± 0.51 for African dust conditions in this location. RF (at shortwave radiation) seems to decrease as the African dust contribution at ground level is larger which indicates the cooling effect of African dust aerosol in Madrid. We have also proved the potential of a 2D-cluster analysis based on AAE and SAE to differentiate both situations in Madrid. Conversely, it is suggested that aerosols observed in La Coruña under dust-free conditions might come from different sources. Then, SAE and AAE are not good enough indicators to distinguish between dust-free and African dust conditions. Besides, as La Coruña is at a further distance

  1. Mineral dust aerosols promote the formation of toxic nitropolycyclic aromatic compounds

    PubMed Central

    Kameda, Takayuki; Azumi, Eri; Fukushima, Aki; Tang, Ning; Matsuki, Atsushi; Kamiya, Yuta; Toriba, Akira; Hayakawa, Kazuichi

    2016-01-01

    Atmospheric nitrated polycyclic aromatic hydrocarbons (NPAHs), which have been shown to have adverse health effects such as carcinogenicity, are formed in part through nitration reactions of their parent polycyclic aromatic hydrocarbons (PAHs) in the atmosphere. However, little is known about heterogeneous nitration rates of PAHs by gaseous NO2 on natural mineral substrates, such as desert dust aerosols. Herein by employing kinetic experiments using a flow reactor and surface analysis by Fourier transform infrared spectroscopy with pyridine adsorption, we demonstrate that the reaction is accelerated on acidic surfaces of mineral dust, particularly on those of clay minerals. In support of this finding, we show that levels of ambient particle-associated NPAHs in Beijing, China, significantly increased during heavy dust storms. These results suggest that mineral dust surface reactions are an unrecognized source of toxic organic chemicals in the atmosphere and that they enhance the toxicity of mineral dust aerosols in urban environments. PMID:27075250

  2. Issues related to dust aerosols in the magnesite industry. I. Chamber exposure.

    PubMed

    Reichrtová, E; Takác, L

    1992-01-01

    The present paper is an overview of the experimental research into the effects of flue magnesite dust in the magnesite industry in which the raw material (magnesite) is processed into refractory magnesite clinker. The issues related to dust are divided into two problem areas: a) dust aerosol arising in the process of ore mining and consisting largely of magnesite (MgCO3) and b) dust aerosol originating during ore baking in rotatory furnaces and made up mostly of MgO. Thus, larger groups of people become exposed to these aerosols as a result of solid particles escaping into the atmosphere than in the case of occupational exposure. Experimental research carried out on laboratory animals after chamber exposure provided findings on the deposition, retention and elimination of magnesite dust, on impaired balance between magnesium and calcium leading to damage of biological membranes, on how the immune profile or reproduction and embryogenesis is impacted as well as on the possible interaction with sodium salicylate as a result of an impaired acid base balance. These findings are followed up by evidence produced in the course of biological monitoring (Part II).

  3. Airborne Sunphotometry of African Dust and Marine Boundary Layer Aerosols in PRIDE

    NASA Technical Reports Server (NTRS)

    Livingston, John M.; Redemann, Jens; Russell, Philip; Schmid, Beat; Reid, Jeff; Pilewskie, Peter; Hipskind, R. Stephen (Technical Monitor)

    2000-01-01

    The Puerto Rico Dust Experiment (PRIDE) was conducted during summer 2000 to study the radiative, microphysical and transport properties of Saharan dust in the Caribbean region. During PRIDE, NASA Ames Research Center's six-channel airborne autotracking sunphotometer (AATS-6) was operated aboard a Piper Navajo airplane based at Roosevelt Roads Naval Station on the northeast coast of Puerto Rico. AATS-6 measurements were taken during 21 science flights off the coast of Puerto Rico in the western Caribbean. Data were acquired within and above the Marine Boundary Layer (MBL) and the Saharan Aerosol Layer (SAL) up to 5.5 km altitude tinder a wide range of dust loadings. Aerosol optical depth (AOD) spectra and columnar water vapor (CWV) values have been calculated from the AATS-6 measurements by using sunphotometer calibration data obtained at Mauna Loa Observatory (3A kin ASL) before (May) and after (October) PRIDE. Mid-visible AOD values measured near the surface during PRIDE ranged from 0.07 on the cleanest day to 0.55 on the most turbid day. Values measured above the MBL were as high as 0.35; values above the SAL were as low as 0.01. The fraction of total column AOD due to Saharan dust cannot be determined precisely from AATS-6 AOD data alone due to the uncertainty in the extent of vertical mixing of the dust down through the MBL. However, analyses of ground-based and airborne in-situ aerosol sampling measurements and ground-based aerosol lidar backscatter data should yield accurate characterization of the vertical mixing that will enable calculation of the Saharan dust AOD component from the sunphotometer data. Examples will be presented showing measured AATS-6 AOD spectra, calculated aerosol extinction and water vapor density vertical profiles, and aerosol size distributions retrieved by inversion of the AOD spectra. Near sea-surface AOD spectra acquired by AATS-6 during horizontal flight legs at 30 m ASL are available for validation of AOD derived from coincident

  4. Light-Absorbing Brown Carbon Aerosol Constituents from Combustion of Indonesian Peat and Biomass.

    PubMed

    Budisulistiorini, Sri Hapsari; Riva, Matthieu; Williams, Michael; Chen, Jing; Itoh, Masayuki; Surratt, Jason D; Kuwata, Mikinori

    2017-04-18

    Light-absorbing brown carbon (BrC) constituents of organic aerosol (OA) have been shown to significantly absorb ultraviolet (UV) and visible light and thus impact radiative forcing. However, molecular identification of the BrC constituents is still limited. In this study, we characterize BrC constituents at the molecular level in (i) aerosols emitted by combustion of peat, fern/leaf, and charcoal from Indonesia and (ii) ambient aerosols collected in Singapore during the 2015 haze episode. Aerosols were analyzed using ultra performance liquid chromatography instrument interfaced to a diode array detector and electrospray ionization high-resolution quadrupole time-of-flight mass spectrometer operated in the negative ion mode. In the laboratory-generated aerosols, we identified 41 compounds that can potentially absorb near-UV and visible wavelengths, such as oxygenated-conjugated compounds, nitroaromatics, and S-containing compounds. The sum of BrC constituents in peat, fern/leaf, and charcoal burning aerosols are 16%, 35%, and 28% of the OA mass, respectively, giving an average contribution of 24%. On average, the BrC constituents account for 0.4% of the ambient OA mass; however, large uncertainties in mass closure remain because of the lack of authentic standards. This study highlights the potential of light-absorbing BrC OA constituents from peat, fern/leaf, and charcoal burning and their importance in the atmosphere.

  5. Nine-year spatial and temporal evolution of desert dust aerosols over South and East Asia as revealed by CALIOP

    NASA Astrophysics Data System (ADS)

    Proestakis, Emmanouil; Amiridis, Vassilis; Marinou, Eleni; Georgoulias, Aristeidis K.; Solomos, Stavros; Kazadzis, Stelios; Chimot, Julien; Che, Huizheng; Alexandri, Georgia; Binietoglou, Ioannis; Daskalopoulou, Vasiliki; Kourtidis, Konstantinos A.; de Leeuw, Gerrit; van der A, Ronald J.

    2018-02-01

    We present a 3-D climatology of the desert dust distribution over South and East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network). The method involves the use of the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, applied to multiyear CALIPSO observations (January 2007-December 2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over South and East Asia along with the seasonal transition of dust transport pathways. Persistent high D_AOD (dust aerosol optical depth) values at 532 nm, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with the highest values observed during spring for northern China (Taklimakan and Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally, we decompose the CALIPSO AOD (aerosol optical depth) into dust and non-dust aerosol components to reveal the non-dust AOD over the highly industrialized and densely populated regions of South and East Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D_AOD time series and trends between January 2007 and December 2015 are calculated over South and East Asia and over selected subregions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China trends are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.

  6. Development of Atmospheric Chemistry-Aerosol Transport Model for Bioavailable Iron From Dust and Combustion Source

    NASA Astrophysics Data System (ADS)

    Ito, A.; Feng, Y.

    2009-12-01

    An accurate prediction of bioavailable iron fraction for ocean biota is hampered by uncertainties in modeling soluble iron fractions in atmospheric aerosols. It has been proposed that atmospheric processing of mineral aerosols by anthropogenic pollutants may be a key pathway to transform insoluble iron into soluble forms. The dissolution of dust minerals strongly depends on solution pH, which is sensitive to the heterogeneous uptake of soluble gases by the dust particle. Due to the complexity, previous model assessments generally use a common assumption in thermodynamical equilibrium between gas and aerosol phases. Here, we compiled an emission inventory of iron from combustion and dust source, and incorporated a dust iron dissolution scheme in a global chemistry-aerosol transport model (IMPACT). We will examine and discuss the uncertainties in estimation of dissolved iron as well as comparisons of the model results with available observations.

  7. Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study

    NASA Astrophysics Data System (ADS)

    Caponi, Lorenzo; Formenti, Paola; Massabó, Dario; Di Biagio, Claudia; Cazaunau, Mathieu; Pangui, Edouard; Chevaillier, Servanne; Landrot, Gautier; Andreae, Meinrat O.; Kandler, Konrad; Piketh, Stuart; Saeed, Thuraya; Seibert, Dave; Williams, Earle; Balkanski, Yves; Prati, Paolo; Doussin, Jean-François

    2017-06-01

    This paper presents new laboratory measurements of the mass absorption efficiency (MAE) between 375 and 850 nm for 12 individual samples of mineral dust from different source areas worldwide and in two size classes: PM10. 6 (mass fraction of particles of aerodynamic diameter lower than 10.6 µm) and PM2. 5 (mass fraction of particles of aerodynamic diameter lower than 2.5 µm). The experiments were performed in the CESAM simulation chamber using mineral dust generated from natural parent soils and included optical and gravimetric analyses. The results show that the MAE values are lower for the PM10. 6 mass fraction (range 37-135 × 10-3 m2 g-1 at 375 nm) than for the PM2. 5 (range 95-711 × 10-3 m2 g-1 at 375 nm) and decrease with increasing wavelength as λ-AAE, where the Ångström absorption exponent (AAE) averages between 3.3 and 3.5, regardless of size. The size independence of AAE suggests that, for a given size distribution, the dust composition did not vary with size for this set of samples. Because of its high atmospheric concentration, light absorption by mineral dust can be competitive with black and brown carbon even during atmospheric transport over heavy polluted regions, when dust concentrations are significantly lower than at emission. The AAE values of mineral dust are higher than for black carbon (˜ 1) but in the same range as light-absorbing organic (brown) carbon. As a result, depending on the environment, there can be some ambiguity in apportioning the aerosol absorption optical depth (AAOD) based on spectral dependence, which is relevant to the development of remote sensing of light-absorbing aerosols and their assimilation in climate models. We suggest that the sample-to-sample variability in our dataset of MAE values is related to regional differences in the mineralogical composition of the parent soils. Particularly in the PM2. 5 fraction, we found a strong linear correlation between the dust light-absorption properties and

  8. Radiative Energetics of Mineral Dust Aerosols from Ground-Based Measurements

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Hansell, Richard A.

    2011-01-01

    Airborne dust aerosols worldwide contribute a significant part to air quality problems and, to some extent, regional climatic issues (e.g., radiative forcing, hydrological cycle, and primary biological productivity in oceans). Evaluating the direct solar radiative effect of dust aerosols is relatively straightforward due in part to the relatively large SIN ratio in broadband irradiance measurements. The longwave (LW) impact, on the other hand, is rather difficult to ascertain since the measured dust signal level (approx.10 W/sq m) is on the same order as the instrumental uncertainties. Although the magnitude of the LW impact is much smaller than that of the shortwave (SW), it can still have a noticeable influence on the energy distribution of Earth-atmosphere system, particularly due to the strong light-absorptive properties commonly found in many terrestrial minerals. The current effort is part of an ongoing research study to perform a global assessment of dust direct aerosol radiative effects (DARE) during major field deployments of key dust source regions worldwide. In this work we present results stemming from two previous field deployments: the 2006 NASA African Monsoon Multidisciplinary Activities and the 2008 Asian Monsoon Years, both utilizing NASA Goddard's mobile ground-based facility. The former study focused on transported Saharan dust at Sal (16.73degN, 22.93degW), Cape Verde along the west coast of Africa while the latter focused on Asian dust at Zhangye (39.082degN, 100.276degE), China near the source between the Taklimakan and Gobi deserts. Due to the compelling variability in spatial and temporal scale of dust properties during field experiments, a deterministic I-D radiative transfer model constrained by local measurements (i.e., spectral photometry/interferometry and lidar for physical/microphysical, mineralogy, and single-scattering properties) is employed to evaluate dust's local instantaneous SW/LW DARE both at the surface and at the top of

  9. Estimation of columnar concentrations of absorbing and scattering fine mode aerosol components using AERONET data

    NASA Astrophysics Data System (ADS)

    Choi, Yongjoo; Ghim, Young Sung

    2016-11-01

    Columnar concentrations of absorbing and scattering components of fine mode aerosols were estimated using Aerosol Robotic Network (AERONET) data for a site downwind of Seoul. The study period was between March 2012 and April 2013 including the period of the Distributed Regional Aerosol Gridded Observation Networks (DRAGON)-Asia campaign in March to May 2012. The Maxwell Garnett mixing rule was assumed for insoluble components embedded in a host solution, while the volume average mixing rule was assumed for the aqueous solution of soluble components. During the DRAGON-Asia campaign the surface concentrations of major components of fine particles were measured. The columnar mass fractions of black carbon (BC), organic carbon (OC), mineral dust (MD), and ammonium sulfate (AS) were 1.5, 5.9, 6.6, and 52%, respectively, which were comparable to the mass fractions measured at the surface for BC, OC, and secondary inorganic aerosols at 2.3, 18, and 55%. The vertical distributions of BC and AS were investigated by employing the concept of a column height. While the column height for BC was similar to the planetary boundary layer (PBL) height, that for AS was 4.4 times higher than the PBL height and increased with air temperature from March to May. The monthly variations of the columnar mass concentrations during the study period were generally well explained in term of meteorology and emission characteristics. However, certain variations of MD were different from those typically observed primarily because only fine mode aerosols were considered.

  10. Water uptake of clay and desert dust aerosol particles at sub- and supersaturated water vapor conditions

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Herich, Hanna; Tritscher, Torsten; Wiacek, Aldona

    2009-11-01

    Airborne mineral dust particles serve as cloud condensation nuclei (CCN), thereby influencing the formation and properties of warm clouds. It is therefore of particular interest how dust aerosols with different mineralogy behave when exposed to high relative humidity (RH) or supersaturation with respect to liquid water similar to atmospheric conditions. In this study the sub-saturated hygroscopic growth and the supersaturated cloud condensation nucleus activity of pure clays and real desert dust aerosols was determined using a hygroscopicity tandem differential mobility analyzer (HTDMA) and a cloud condensation nuclei counter (CCNC), respectively. Five different illite, montmorillonite and kaolinite clay samples as wellmore » as three desert dust samples (Saharan dust (SD), Chinese dust (CD) and Arizona test dust (ATD)) were used. Aerosols were generated both with a wet and a dry disperser and the water uptake was parameterized via the hygroscopicity parameter, κ. The hygroscopicity of dry generated dust aerosols was found to be negligible when compared to processed atmospheric aerosols, with CCNC derived κ values between 0.00 and 0.02. The latter value can be idealized as a particle consisting of 96.7% (by volume) insoluble material and ~3.3% ammonium sulfate. Pure clay aerosols were found to be generally less hygroscopic than real desert dust particles. All illite and montmorillonite samples had κ~0.003, kaolinites were least hygroscopic and had κ=0.001. SD (κ=0.023) was found to be the most hygroscopic dry-generated desert dust followed by CD (κ=0.007) and ATD (κ=0.003). Wet-generated dust showed an increased water uptake when compared to dry-generated samples. This is considered to be an artifact introduced by redistribution of soluble material between the particles while immersed in an aqueous medium during atomization, thus indicating that specification of the generation method is critically important when presenting such data. Any atmospheric

  11. Water uptake of clay and desert dust aerosol particles at sub- and supersaturated water vapor conditions.

    PubMed

    Herich, Hanna; Tritscher, Torsten; Wiacek, Aldona; Gysel, Martin; Weingartner, Ernest; Lohmann, Ulrike; Baltensperger, Urs; Cziczo, Daniel J

    2009-09-28

    Airborne mineral dust particles serve as cloud condensation nuclei (CCN), thereby influencing the formation and properties of warm clouds. It is therefore of atmospheric interest how dust aerosols with different mineralogy behave when exposed to high relative humidity (RH) or supersaturation (SS) with respect to liquid water. In this study the subsaturated hygroscopic growth and the supersaturated cloud condensation nucleus activity of pure clays and real desert dust aerosols were determined using a hygroscopicity tandem differential mobility analyzer (HTDMA) and a cloud condensation nuclei counter (CCNC), respectively. Five different illite, montmorillonite and kaolinite clay samples as well as three desert dust samples (Saharan dust (SD), Chinese dust (CD) and Arizona test dust (ATD)) were investigated. Aerosols were generated both with a wet and a dry disperser. The water uptake was parameterized via the hygroscopicity parameter kappa. The hygroscopicity of dry generated dust aerosols was found to be negligible when compared to processed atmospheric aerosols, with CCNC derived kappa values between 0.00 and 0.02 (the latter corresponds to a particle consisting of 96.7% by volume insoluble material and approximately 3.3% ammonium sulfate). Pure clay aerosols were generally found to be less hygroscopic than natural desert dust particles. The illite and montmorillonite samples had kappa approximately 0.003. The kaolinite samples were less hygroscopic and had kappa=0.001. SD (kappa=0.023) was found to be the most hygroscopic dry-generated desert dust followed by CD (kappa=0.007) and ATD (kappa=0.003). Wet-generated dust showed an increased water uptake when compared to dry-generated samples. This is considered to be an artifact introduced by redistribution of soluble material between the particles. Thus, the generation method is critically important when presenting such data. These results indicate any atmospheric processing of a fresh mineral dust particle which

  12. The Impact of Desert Dust Aerosol Radiative Forcing on Global and West African Precipitation

    NASA Astrophysics Data System (ADS)

    Jordan, A.; Zaitchik, B. F.; Gnanadesikan, A.; Dezfuli, A. K.

    2015-12-01

    Desert dust aerosols exert a radiative forcing on the atmosphere, influencing atmospheric temperature structure and modifying radiative fluxes at the top of the atmosphere (TOA) and surface. As dust aerosols perturb radiative fluxes, the atmosphere responds by altering both energy and moisture dynamics, with potentially significant impacts on regional and global precipitation. Global Climate Model (GCM) experiments designed to characterize these processes have yielded a wide range of results, owing to both the complex nature of the system and diverse differences across models. Most model results show a general decrease in global precipitation, but regional results vary. Here, we compare simulations from GFDL's CM2Mc GCM with multiple other model experiments from the literature in order to investigate mechanisms of radiative impact and reasons for GCM differences on a global and regional scale. We focus on West Africa, a region of high interannual rainfall variability that is a source of dust and that neighbors major Sahara Desert dust sources. As such, changes in West African climate due to radiative forcing of desert dust aerosol have serious implications for desertification feedbacks. Our CM2Mc results show net cooling of the planet at TOA and surface, net warming of the atmosphere, and significant increases in precipitation over West Africa during the summer rainy season. These results differ from some previous GCM studies, prompting comparative analysis of desert dust parameters across models. This presentation will offer quantitative analysis of differences in dust aerosol parameters, aerosol optical properties, and overall particle burden across GCMs, and will characterize the contribution of model differences to the uncertainty of forcing and climate response affecting West Africa.

  13. Optical properties of mineral dust aerosol in the thermal infrared

    NASA Astrophysics Data System (ADS)

    Köhler, Claas H.

    2017-02-01

    The optical properties of mineral dust and biomass burning aerosol in the thermal infrared (TIR) are examined by means of Fourier Transform Infrared Spectrometer (FTIR) measurements and radiative transfer (RT) simulations. The measurements were conducted within the scope of the Saharan Mineral Dust Experiment 2 (SAMUM-2) at Praia (Cape Verde) in January and February 2008. The aerosol radiative effect in the TIR atmospheric window region 800-1200 cm-1 (8-12 µm) is discussed in two case studies. The first case study employs a combination of IASI measurements and RT simulations to investigate a lofted optically thin biomass burning layer with emphasis on its potential influence on sea surface temperature (SST) retrieval. The second case study uses ground based measurements to establish the importance of particle shape and refractive index for benchmark RT simulations of dust optical properties in the TIR domain. Our research confirms earlier studies suggesting that spheroidal model particles lead to a significantly improved agreement between RT simulations and measurements compared to spheres. However, room for improvement remains, as the uncertainty originating from the refractive index data for many aerosol constituents prohibits more conclusive results.

  14. Vertical Profiles of Light-Absorbing Aerosol: A Combination of In-situ and AERONET Observations during NASA DISCOVER-AQ

    NASA Astrophysics Data System (ADS)

    Ziemba, L. D.; Beyersdorf, A. J.; Chen, G.; Corr, C.; Crumeyrolle, S.; Giles, D. M.; Holben, B. N.; Hudgins, C.; Martin, R.; Moore, R.; Shook, M.; Thornhill, K. L., II; Winstead, E.; Anderson, B. E.

    2014-12-01

    Understanding the vertical profile of atmospheric aerosols plays a vital role in utilizing spaceborne, column-integrated satellite observations. The properties and distribution of light-absorbing aerosol are particularly uncertain despite significant air quality and climate ramifications. Advanced retrieval algorithms are able to derive complex aerosol properties (e.g., wavelength-dependent absorption coefficient and single scattering albedo) from remote-sensing measurements, but quantitative relationships to surface conditions remain a challenge. Highly systematic atmospheric profiling during four unique deployments for the NASA DISCOVER-AQ project (Baltimore, MD, 2011; San Joaquin Valley, CA, 2013; Houston, TX, 2013; Denver, CO, 2014) allow statistical assessment of spatial, temporal, and source-related variability for light-absorbing aerosol properties in these distinct regions. In-situ sampling in conjunction with a dense network of AERONET sensors also allows evaluation of the sensitivity, limitations, and advantages of remote-sensing data products over a wide range of conditions. In-situ aerosol and gas-phase observations were made during DISCOVER-AQ aboard the NASA P-3B aircraft. Aerosol absorption coefficients were measured by a Particle Soot Absorption Photometer (PSAP). Approximately 200 profiles for each of the four deployments were obtained, from the surface (25-300m altitude) to 5 km, and are used to calculate absorption aerosol optical depths (AAODs). These are quantitatively compared to AAOD derived from AERONET Level 1.5 retrievals to 1) explore discrepancies between measurements, 2) quantify the fraction of AAOD that exists directly at the surface and is often missed by airborne sampling, and 3) evaluate the potential for deriving ground-level black carbon (BC) concentrations for air quality prediction. Aerosol size distributions are used to assess absorption contributions from mineral dust, both at the surface and aloft. SP2 (Single Particle Soot

  15. Uptake of Nitrate and Sulfate on Dust Aerosols during TRACE-P

    NASA Technical Reports Server (NTRS)

    Jordan, C. E.; Dibb, J. E.; Anderson, B. E.; Fuelberg, H. E.

    2003-01-01

    Aerosol data collected near Asia on the DC-8 aircraft platform during TRACE-P has been examined for evidence of uptake of NO3(-) and SO4(-) on dust surfaces. Data is compared between a sector where dust was predominant and a sector where dust was less of an influence. Coincident with dust were higher mixing ratios of anthropogenic pollutants. HNO3, SO2, and CO were higher in the dust sector than the nondust sector by factors of 2.7, 6.2, and 1.5, respectively. The colocation of dust and pollution sources allowed for the uptake of NO3(-) and nss-SO4(-) on the coarse dust aerosols, increasing the mixing ratios of these particulates by factors of 5.7 and 2.6 on average. There was sufficient nss-SO4(-) to take up all of the NH4(+) present, with enough excess nss-SO4(-) to also react with dust CaCO3. This suggests that the enhanced NO3(-) was not in fine mode NH4NO3. Particulate NO3(-) (p-NO3(-)) constituted 54% of the total NO3(-), (t-NO3(-)) on average, reaching a maximum of 72% in the dust sector. In the nondust sector, p-NO3(-) contributed 37% to t-NO3(-), likely due to the abundance of sea salts there. In two other sectors where the influence of dust and sea salt were minimal, p-NO3(-), accounted for < 15% of t-NO3(-).

  16. Optical and microphysical properties of natural mineral dust and anthropogenic soil dust near dust source regions over northwestern China

    NASA Astrophysics Data System (ADS)

    Wang, Xin; Wen, Hui; Shi, Jinsen; Bi, Jianrong; Huang, Zhongwei; Zhang, Beidou; Zhou, Tian; Fu, Kaiqi; Chen, Quanliang; Xin, Jinyuan

    2018-02-01

    Mineral dust aerosols (MDs) not only influence the climate by scattering and absorbing solar radiation but also modify cloud properties and change the ecosystem. From 3 April to 16 May 2014, a ground-based mobile laboratory was deployed to measure the optical and microphysical properties of MDs near dust source regions in Wuwei, Zhangye, and Dunhuang (in chronological order) along the Hexi Corridor over northwestern China. Throughout this dust campaign, the hourly averaged (±standard deviation) aerosol scattering coefficients (σsp, 550 nm) of the particulates with aerodynamic diameters less than 2.5 µm (PM2.5) at these three sites were sequentially 101.5 ± 36.8, 182.2 ± 433.1, and 54.0 ± 32.0 Mm-1. Correspondingly, the absorption coefficients (σap, 637 nm) were 9.7 ± 6.1, 6.0 ± 4.6, and 2.3 ± 0.9 Mm-1; single-scattering albedos (ω, 637 nm) were 0.902 ± 0.025, 0.931 ± 0.037, and 0.949 ± 0.020; and scattering Ångström exponents (Åsp, 450-700 nm) of PM2.5 were 1.28 ± 0.27, 0.77 ± 0.51, and 0.52 ± 0.31. During a severe dust storm in Zhangye (i.e., from 23 to 25 April), the highest values of σsp2.5 ( ˜ 5074 Mm-1), backscattering coefficient (σbsp2.5, ˜ 522 Mm-1), and ω637 ( ˜ 0.993) and the lowest values of backscattering fraction (b2.5, ˜ 0.101) at 550 nm and Åsp2.5 ( ˜ -0.046) at 450-700 nm, with peak values of aerosol number size distribution (appearing at the particle diameter range of 1-3 µm), exhibited that the atmospheric aerosols were dominated by coarse-mode dust aerosols. It is hypothesized that the relatively higher values of mass scattering efficiency during floating dust episodes in Wuwei and Zhangye are attributed to the anthropogenic soil dust produced by agricultural cultivations.

  17. Effects of Aerosol on Atmospheric Dynamics and Hydrologic Processes During Boreal Spring and Summer

    NASA Technical Reports Server (NTRS)

    Lau, William K. M.; Kim, M. K.; Kim, K. M.; Chin, Mian

    2005-01-01

    Global and regional climate impacts of present-day aerosol loading during boreal spring are investigated using the NASA finite volume General Circulation Model (fvGCM). Three-dimensional distributions of loadings of five species of tropospheric aerosols, i.e., sulfate, black carbon, organic carbon, soil dust, and sea salt are prescribed from outputs of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol loadings are used to calculate the extinction coefficient, single scattering albedo, and asymmetric factor at eleven spectral wavelengths in the radiative transfer code. We find that aerosol-radiative forcing during boreal spring excites a wavetrain-like pattern in tropospheric temperature and geopotential height that emanates from Northern Africa, through Eurasia, to northeastern Pacific. Associated with the teleconnection is strong surface cooling over regions with large aerosol loading, i.e., China, India, and Africa. Low-to-mid tropospheric heating due to shortwave absorption is found in regions with large loading of dust (Northern Africa, and central East Asia), and black carbon (South and East Asia). In addition pronounced surface cooling is found over the Caspian Sea and warming over Eurasian and northeastern Asia, where aerosol loadings are relatively low. These warming and cooling are components of teleconnection pattern produced primarily by atmospheric heating from absorbing aerosols, i.e., dust from North Africa and black carbon from South and East Asia. Effects of aerosols on atmospheric hydrologic cycle in the Asian monsoon region are also investigated. Results show that absorbing aerosols, i.e., black carbon and dust, induce large-scale upper-level heating anomaly over the Tibetan Plateau in April and May, ushering in an early onset of the Indian summer monsoon. Absorbing aerosols also enhance lower-level heating and anomalous ascent over northern India, intensifying the Indian monsoon. Overall, the aerosol

  18. Effects of Aerosol on Atmospheric Dynamics and Hydrologic Processes during Boreal Spring and Summer

    NASA Technical Reports Server (NTRS)

    Lau, William K. M.; Kim, M. K.; Chin, Mian; Kim, K. M.

    2005-01-01

    Global and regional climate impacts of present-day aerosol loading during boreal spring are investigated using the NASA finite volume General Circulation Model (fvGCM). Three-dimensional distributions of loadings of five species of tropospheric aerosols, i.e., sulfate, black carbon, organic carbon, soil dust, and sea salt are prescribed from outputs of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol loadings are used to calculate the extinction coefficient, single scattering albedo, and asymmetric factor at eleven spectral wavelengths in the radiative transfer code. We find that aerosol-radiative forcing during boreal spring excites a wavetrain-like pattern in tropospheric temperature and geopotential height that emanates from Northern Africa, through Eurasia, to northeastern Pacific. Associated with the teleconnection is strong surface cooling over regions with large aerosol loading, i.e., China, India, and Africa. Low-to-mid tropospheric heating due to shortwave absorption is found in regions with large loading of dust (Northern Africa, and central East Asia), and black carbon (South and East Asia). In addition pronounced surface cooling is found over the Caspian Sea and warming over Eurasian and northeastern Asia, where aerosol loadings are relatively low. These warming and cooling are components of teleconnection pattern produced primarily by atmospheric heating from absorbing aerosols, i.e., dust from North Africa and.black carbon from South and East Asia. Effects of aerosols on atmospheric hydrologic cycle in the Asian monsoon region are also investigated. Results show that absorbing aerosols, i.e., black carbon and dust, induce large-scale upper-level heating anomaly over the Tibetan Plateau in April and May, ushering in an early onset of the Indian summer monsoon. Absorbing aerosols also enhance lower-level heating and anomalous ascent over northern India, intensifying the Indian monsoon. Overall, the aerosol

  19. AERONET-Based Nonspherical Dust Optical Models and Effects on the VIIRS Deep Blue/SOAR Over Water Aerosol Product

    NASA Astrophysics Data System (ADS)

    Lee, Jaehwa; Hsu, N. Christina; Sayer, Andrew M.; Bettenhausen, Corey; Yang, Ping

    2017-10-01

    Aerosol Robotic Network (AERONET)-based nonspherical dust optical models are developed and applied to the Satellite Ocean Aerosol Retrieval (SOAR) algorithm as part of the Version 1 Visible Infrared Imaging Radiometer Suite (VIIRS) NASA "Deep Blue" aerosol data product suite. The optical models are created using Version 2 AERONET inversion data at six distinct sites influenced frequently by dust aerosols from different source regions. The same spheroid shape distribution as used in the AERONET inversion algorithm is assumed to account for the nonspherical characteristics of mineral dust, which ensures the consistency between the bulk scattering properties of the developed optical models and the AERONET-retrieved microphysical and optical properties. For the Version 1 SOAR aerosol product, the dust optical model representative for Capo Verde site is used, considering the strong influence of Saharan dust over the global ocean in terms of amount and spatial coverage. Comparisons of the VIIRS-retrieved aerosol optical properties against AERONET direct-Sun observations at five island/coastal sites suggest that the use of nonspherical dust optical models significantly improves the retrievals of aerosol optical depth (AOD) and Ångström exponent by mitigating the well-known artifact of scattering angle dependence of the variables, which is observed when incorrectly assuming spherical dust. The resulting removal of these artifacts results in a more natural spatial pattern of AOD along the transport path of Saharan dust to the Atlantic Ocean; that is, AOD decreases with increasing distance transported, whereas the spherical assumption leads to a strong wave pattern due to the spurious scattering angle dependence of AOD.

  20. Natural and Anthropogenic Aerosols in the World's Megacities and Climate Impacts

    NASA Astrophysics Data System (ADS)

    Kafatos, M.; Singh, R.; El-Askary, H.; Qu, J.

    2005-12-01

    aerosols. The highest boundary layer heights are associated with regions where the sensible heat flux is greatest, and latent heat flux is smallest due to lack of vegetation. Boundary layer heights in the deserts may be systematically higher than the slightly wetter regions at the edges of deserts. Latent heat flux model runs and MODIS observations of dust storms affecting the Nile Delta and Cairo indicate strong influence on the local weather and climate forcings. In the Indo-Gangetic, during the pre-monsoon period, dust storms form. We have examined SDS transport using RS data acquired from NASA's MODIS MISR instruments and from sun photometer measurements. The aerosol optical depth and size of the dust particles are found to be significantly higher during such dust storm events. Moreover, our results clearly show that power plants in this region are the key point source of air pollutants. The detailed analysis of aerosol parameters show the existence of absorbing and non-absorbing aerosols emitted from these plants. The combined effects of urban aerosols with dust aerosols in India and Cairo not only affect megacities, they also have long-term climate impacts. We will also discuss how the assimilation of RS data into mesoscale models can improve these models and predictability of hazards and effects on megacities, such as SDS events, and forest fires, all sources of aerosols. Therefore RS data can improve the prediction of climate forcings by aerosols.

  1. Using the OMI Aerosol Index and Absorption Aerosol Optical Depth to evaluate the NASA MERRA Aerosol Reanalysis

    NASA Astrophysics Data System (ADS)

    Buchard, V.; da Silva, A. M.; Colarco, P. R.; Darmenov, A.; Randles, C. A.; Govindaraju, R.; Torres, O.; Campbell, J.; Spurr, R.

    2014-12-01

    A radiative transfer interface has been developed to simulate the UV Aerosol Index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and Aerosol Absorption Optical Depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of Aerosol Optical Depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the Aerosol Robotic Network (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the South African and South American biomass burning regions indicates that revising the spectrally-dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons

  2. Using the OMI aerosol index and absorption aerosol optical depth to evaluate the NASA MERRA Aerosol Reanalysis

    NASA Astrophysics Data System (ADS)

    Buchard, V.; da Silva, A. M.; Colarco, P. R.; Darmenov, A.; Randles, C. A.; Govindaraju, R.; Torres, O.; Campbell, J.; Spurr, R.

    2015-05-01

    A radiative transfer interface has been developed to simulate the UV aerosol index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and aerosol absorption optical depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the AErosol RObotic NETwork (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model-produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the southern African and South American biomass burning regions indicates that revising the spectrally dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons

  3. The climate impacts of absorbing aerosols on and within the Arctic

    NASA Astrophysics Data System (ADS)

    Rasch, P.; Wang, H.; Ma, P.; Fast, J. D.; Wang, M.; Easter, R. C.; Liu, X.; Qian, Y.; Flanner, M. G.; Ghan, S.; Singh, B.

    2011-12-01

    Absorbing aerosols are receiving increasing attention as forcing agents in the climate system. By scattering and absorbing light they can reduce planetary albedo, particularly over bright surfaces (clouds, snow and ice). They also act as cloud condensation and/or ice nuclei, influencing the brightness, lifetime and precipitation properties of clouds. Atmospheric stability and primary circulation features respond to the changing vertical and horizontal patterns of heating, cooling, and surface fluxes produced by the aerosols, clouds and surface properties. These changes in meteorology have further impacts on aerosols and clouds producing a complex interplay between transport, forcings, and feedbacks involving absorbing aerosols and climate. The complexity of the processes and the interactions between them make it very challenging to represent aerosols realistically in large scale (global and regional) climate models. Simulations of important features of aerosols still contain easily identifiable biases. I will describe our efforts to identify the processes responsible for some of those biases and the deficiencies in model formulations that impede progress in treating aerosols and understanding their role in polar climate. I plan to summarize some studies performed with the NCAR CESM (global) and WRF-Chem (regional) Community models that examine the simulation sensitivity to treatments of physics, chemistry, and meteorology. Some of these simulations were allowed to evolve freely; others were strongly constrained to agree with observed meteorological fields. We have also altered the formulation of a number of the processes in the model to improve fidelity in the aerosol distributions. The parameterizations used in our global model have also been transferred to the regional model, allowing comparisons to be made between the simpler formulations used in the global model with more elaborate and costly formulations available in the regional model. The regional model can

  4. African aerosols and Atlantic tropical cyclone activities

    NASA Astrophysics Data System (ADS)

    Kafatos, M.; Sun, D.; Sahoo, A.

    2006-12-01

    Previous studies have shown that the Atlantic basin major hurricane (MH) activity is associated with western Sahelian monsoon rainfall, while rainfall in the Sahel is found to be highly anti-correlated with the African dust storms. So if the Atlantic basin MH activity may be anti-correlated with the African dust aerosols? In order to investigate the relationship between the African dust and the tropical cyclone (including both tropical storms and hurricanes) activities in the Atlantic basin, we explore how the African dust may link to Atlantic TC activity by using the long-term (1982-2005) NCEP Reynolds sea surface temperature (SST) product, and tropical cyclone (TC) data from the National Hurricane Center Best Track Files, and the TOMS aerosol index (AI) data, because the TOMS AI positive values are associated with UV-absorbing aerosols, like dust and smoke. Although no significant negative correlation between the TOMS AI and the Atlantic TC or MH frequency and duration is found, the initial locations of the Atlantic tropical cyclones did occur over the ocean where the aerosol loading was low. Our analysis shows that SST over the north tropical Atlantic ocean is anti-correlated with the TOMS aerosol index. This may be due to the radiative forcing of the aerosols. The effects of the dust aerosols carried across the West African region led to a lowering of SST and therefore inhibited tropical cyclogenesis. During 2005, the aerosol loading along the western African coast was unusually low, while the SST over the main development region (MDR) was abnormally high, and the Atlantic TC/hurricane activities became record strong. We propose future observations to test these results.

  5. Absorbing aerosols facilitate transition of Indian monsoon breaks to active spells

    NASA Astrophysics Data System (ADS)

    Manoj, M. G.; Devara, P. C. S.; Safai, P. D.; Goswami, B. N.

    2011-12-01

    While some long breaks of monsoon intraseasonal oscillations (MISOs) are followed by active spells (BFA), some others are not (BNFA). The circulation during BFA (BNFA) cases helps (prevents) accumulation of absorbing aerosols over central India (CI) resulting in almost three times larger Aerosol Index (AI) over CI, during BFA cases compared to BNFA cases. A seminal role played by the absorbing aerosols in the transition from break to active spells is unraveled through modification of the north-south temperature gradient at lower levels. The meridional gradient of temperature at low level (∆ T) between aerosol-rich CI and pristine equatorial Indian Ocean is large (>6°C) and sustains for long time (>10 days) during BFA leading to significant moisture convergence to CI. The stability effect arising from surface cooling by the aerosols is overcome by the enhanced moisture convergence creating a moist static unstable atmosphere conducive for the large-scale organized convection over the CI region leading to the resurgence of active spells. The moisture convergence induced by ∆ T was also able to overcome possible aerosol indirect effect (Twomey effect) and initiate deep convection and transition to active condition. During BNFA cases, however the maximum ∆ T, which was weaker than the BFA cases by more than 1.5°C, could not sustain required moisture convergence and failed to lead to a sustained active spell. Using data from MODIS (MODerate resolution Imaging Spectroradiometer) onboard Terra and several other input parameters from various satellites for the period 2000-2009, the aerosol induced radiative forcing representative of two regions—the CI to the north and the pristine ocean to the south—were estimated and support the differences in observed ∆ T during the two cases. Our results highlight the need for proper inclusion of absorbing aerosols in dynamical models for simulation of the observed variability of MISOs and their extended range prediction.

  6. Retrieving the Height of Smoke and Dust Aerosols by Synergistic Use of Multiple Satellite Sensors

    NASA Technical Reports Server (NTRS)

    Lee, Jaehwa; Hsu, N. Christina; Bettenhausen, Corey; Sayer, Andrew M.; Seftor, Colin J.; Jeong, Myeong-Jae

    2016-01-01

    The Aerosol Single scattering albedo and Height Estimation (ASHE) algorithm was first introduced in Jeong and Hsu (2008) to provide aerosol layer height and single scattering albedo (SSA) for biomass burning smoke aerosols. By using multiple satellite sensors synergistically, ASHE can provide the height information over much broader areas than lidar observations alone. The complete ASHE algorithm uses aerosol data from MODIS or VIIRS, OMI or OMPS, and CALIOP. A simplified algorithm also exists that does not require CALIOP data as long as the SSA of the aerosol layer is provided by another source. Several updates have recently been made: inclusion of dust layers in the retrieval process, better determination of the input aerosol layer height from CALIOP, improvement in aerosol optical depth (AOD) for nonspherical dust, development of quality assurance (QA) procedure, etc.

  7. Desert Dust Layers Over Polluted Marine Boundary Layers: ACE-2 Measurements and ACE-Asia Plans

    NASA Technical Reports Server (NTRS)

    Russell, Philip B.; Schmid, B.; Livingston, J. M.; Redemann, J.; Bergstrom, R. W.; Condon, Estelle P. (Technical Monitor)

    2000-01-01

    Aerosols in ACE-Asia are expected to have some commonalties with those in ACE-2, along with important differences. Among the commonalities are occurrences of desert dust layers over polluted marine boundary layers. Differences include the nature of the dust (yellowish in the East Asia desert outflow, vs. reddish-brown in the Sahara Outflow measured in ACE-2) and the composition of boundary-layer aerosols (e.g., more absorbing, soot and organic aerosol in-the Asian plume, caused by coal and biomass burning, with limited controls). In this paper we present ACE-2 measurements and analyses as a guide to our plans for ACE-2 Asia. The measurements include: (1) Vertical profiles of aerosol optical depth and extinction (380-1558 nm), and of water vapor column and concentration, from the surface through the elevated desert dust, measured by the 14-channel Ames Airborne Tracking Sunphotometer (AATS-14); (2) Comparisons of airborne and shipborne sunphotometer optical depths to satellite-retrieved values, with and without desert dust; (3) Comparisons between airborne Sunphotometer optical depth and extinction spectra and those derived from coincident airborne in situ measurements of aerosol size distribution, scattering and absorption; (4) Comparisons between size distributions measured in situ and retrieved from sunphotometer optical depth spectra; (5) Comparisons between aerosol single scattering albedo values obtained by several techniques, using various combinations of measurements of backscatter, extinction, size distribution, scattering, absorption, and radiative flux. We show how analyses of these data can be used to address questions important to ACE-Asia, such as: (1) How do dust and other absorbing aerosols affect the accuracy of satellite optical depth retrievals? How important are asphericity effects? (2) How important are supermicron dust and seasalt aerosols to overall aerosol optical depth and radiative forcing? How well are these aerosols sampled by aircraft

  8. Critical Reflectance Derived from MODIS: Application for the Retrieval of Aerosol Absorption over Desert Regions

    NASA Technical Reports Server (NTRS)

    Wells, Kelley C.; Martins, J. Vanderlei; Remer, Lorraine A.; Kreidenweis, Sonia M.; Stephens, Graeme L.

    2012-01-01

    Aerosols are tiny suspended particles in the atmosphere that scatter and absorb sunlight. Smoke particles are aerosols, as are sea salt, particulate pollution and airborne dust. When you look down at the earth from space sometimes you can see vast palls of whitish smoke or brownish dust being transported by winds. The reason that you can see these aerosols is because they are reflecting incoming sunlight back to the view in space. The reason for the difference in color between the different types of aerosol is that the particles arc also absorbing sunlight at different wavelengths. Dust appears brownish or reddish because it absorbs light in the blue wavelengths and scatters more reddish light to space, Knowing how much light is scattered versus how much is absorbed, and knowin that as a function of wavelength is essential to being able to quantify the role aerosols play in the energy balance of the earth and in climate change. It is not easy measuring the absorption properties of aerosols when they are suspended in the atmosphere. People have been doing this one substance at a time in the laboratory, but substances mix when they are in the atmosphere and the net absorption effect of all the particles in a column of air is a goal of remote sensing that has not yet been completely successful. In this paper we use a technique based on observing the point at which aerosols change from brightening the surface beneath to darkening it. If aerosols brighten a surface. they must scatter more light to space. If they darken the surface. they must be absorbing more. That cross over point is called the critical reflectance and in this paper we show that critical reflectance is a monotonic function of the intrinsic absorption properties of the particles. This parameter we call the single scattering albedo. We apply the technique to MODIS imagery over the Sahara and Sahel regions to retrieve the single scattering albedo in seven wavelengths, compare these retrievals to ground

  9. Predicting the mineral composition of dust aerosols - Part 1: Representing key processes

    NASA Astrophysics Data System (ADS)

    Perlwitz, J. P.; Pérez García-Pando, C.; Miller, R. L.

    2015-02-01

    Soil dust aerosols created by wind erosion are typically assigned globally uniform physical and chemical properties within Earth system models, despite known regional variations in the mineral content of the parent soil. Mineral composition of the aerosol particles is important to their interaction with climate, including shortwave absorption and radiative forcing, nucleation of cloud droplets and ice crystals, coating by heterogeneous uptake of sulfates and nitrates, and atmospheric processing of iron into bioavailable forms that increase the productivity of marine phytoplankton. Here, aerosol mineral composition is derived by extending a method that provides the composition of a wet-sieved soil. The extension accounts for measurements showing significant differences between the mineral fractions of the wet-sieved soil and the resulting aerosol concentration. For example, some phyllosilicate aerosols are more prevalent at silt sizes, even though they are nearly absent in a soil whose aggregates are dispersed by wet sieving during analysis. We reconstruct the undispersed size distribution of the original soil that is subject to wind erosion. An empirical constraint upon the relative emission of clay and silt is applied that further differentiates the soil and aerosol mineral composition. In addition, a method is proposed for mixing minerals with small impurities composed of iron oxides. These mixtures are important for transporting iron far from the dust source, because pure iron oxides are more dense and vulnerable to gravitational removal than most minerals comprising dust aerosols. A limited comparison to measurements from North Africa shows that the extension brings the model into better agreement, consistent with a more extensive comparison to global observations as well as measurements of elemental composition downwind of the Sahara, as described in companion articles.

  10. Numerical investigation of the coagulation mixing between dust and hygroscopic aerosol particles and its impacts

    NASA Astrophysics Data System (ADS)

    Tsai, I.-Chun; Chen, Jen-Ping; Lin, Yi-Chiu; Chung-Kuang Chou, Charles; Chen, Wei-Nai

    2015-05-01

    A statistical-numerical aerosol parameterization was incorporated into the Community Multiscale Air Quality modeling system to study the coagulation mixing process focusing on a dust storm event that occurred over East Asia. Simulation results show that the coagulation mixing process tends to decrease aerosol mass, surface area, and number concentrations over the dust source areas. Over the downwind oceanic areas, aerosol concentrations generally increased due to enhanced sedimentation as particles became larger upon coagulation. The mixture process can reduce the overall single-scattering albedo by up to 10% as a result of enhanced core with shell absorption by dust and reduction in the number of scattering particles. The enhanced dry deposition speed also altered the vertical distribution. In addition, the ability of aerosol particles to serve as cloud condensation nuclei (CCN) increased from around 107 m-3 to above 109 m-3 over downwind areas because a large amount of mineral dust particles became effective CCN with solute coating, except over the highly polluted areas where multiple collections of hygroscopic particles by dust in effect reduced CCN number. This CCN effect is much stronger for coagulation mixing than by the uptake of sulfuric acid gas on dust, although the nitric acid gas uptake was not investigated. The ability of dust particles to serve as ice nuclei may decrease or increase at low or high subzero temperatures, respectively, due to the switching from deposition nucleation to immersion freezing or haze freezing.

  11. Effects of Absorbing Aerosols on Accelerated Melting of Snowpack in the Hindu-Kush-Himalayas-Tibetan Plateau Region

    NASA Technical Reports Server (NTRS)

    Lau, William K.; Kyu-Myong, Kim; Yasunari, Teppei; Gautam, Ritesh; Hsu, Christina

    2011-01-01

    The impacts of absorbing aerosol on melting of snowpack in the Hindu-Kush-Himalayas-Tibetan Plateau (HKHT) region are studied using in-situ, satellite observations, and GEOS-5 GCM. Based on atmospheric black carbon measurements from the Pyramid observation ( 5 km elevation) in Mt. Everest, we estimate that deposition of black carbon on snow surface will give rise to a reduction in snow surface albedo of 2- 5 %, and an increased annual runoff of 12-34% for a typical Tibetan glacier. Examination of satellite reflectivity and re-analysis data reveals signals of possible impacts of dust and black carbon in darkening the snow surface, and accelerating spring melting of snowpack in the HKHT, following a build-up of absorbing aerosols in the Indo-Gangetic Plain. Results from GCM experiments show that 8-10% increase in the rate of melting of snowpack over the western Himalayas and Tibetan Plateau can be attributed to the elevated-heat-pump (EHP) feedback effect, initiated from the absorption of solar radiation by dust and black carbon accumulated to great height ( 5 km) over the Indo-Gangetic Plain and Himalayas foothills in the pre-monsoon season (April-May). The accelerated melting of the snowpack is enabled by an EHP-induced atmosphere-land-snowpack positive feedback involving a) orographic forcing of the monsoon flow by the complex terrain, and thermal forcing of the HKHT region, leading to increased moisture, cloudiness and rainfall over the Himalayas foothills and northern India, b) warming of the upper troposphere over the Tibetan Plateau, and c) an snow albedo-temperature feedback initiated by a transfer of latent and sensible heat from a warmer atmosphere over the HKHT to the underlying snow surface. Results from ongoing modeling work to assess the relative roles of EHP vs. snow-darkening effects on accelerated melting of snowpack in HKHT region will also be discussed.

  12. Evaluation of the MODIS Retrievals of Dust Aerosol over the Ocean during PRIDE

    NASA Technical Reports Server (NTRS)

    Levy, Robert C.; Remer, Lorraine A.; Tanre, Didier; Kaufman, Yoram J.; Ichoku, Charles; Holben, Brent N.; Livingston, John M.; Russell, Philip B.; Maring, Hal

    2002-01-01

    The Puerto Rico Dust Experiment (PRIDE) took place in Roosevelt Roads, Puerto Rico from June 26 to July 24,2000 to study the radiative and physical properties of African dust aerosol transported into the region. PRIDE had the unique distinction of being the first major field experiment to allow direct comparison of aerosol retrievals from the MODerate Imaging Spectro-radiometer (MODIS) with sunphotometer and in-situ aerosol measurements. Over the ocean, the MODIS algorithm retrieves aerosol optical depth (AOD) as well as information about the aerosols size distribution. During PRIDE, MODIS derived AODs in the red wavelengths (0.66 micrometers) compare closely with AODs measured from sunphotometers, but, are too large at blue and green wavelengths (0.47 and 0.55 micrometers) and too small in the infrared (0.87 micrometers). This discrepancy of spectral slope results in particle size distributions retrieved by MODIS that are small compared to in-situ measurements, and smaller still when compared to sunphotometer sky radiance inversions. The differences in size distributions are, at least in part, associated with MODIS simplification of dust as spherical particles. Analysis of this PRIDE data set is a first step towards derivation of realistic non-spherical models for future MODIS retrievals.

  13. Separating Dust Mixtures and Other External Aerosol Mixtures Using Airborne High Spectral Resolution Lidar Data

    NASA Astrophysics Data System (ADS)

    Burton, S. P.; Ferrare, R. A.; Vaughan, M.; Hostetler, C. A.; Rogers, R. R.; Hair, J. W.; Cook, A. L.; Harper, D. B.

    2013-12-01

    Knowledge of aerosol type is important for source attribution and for determining the magnitude and assessing the consequences of aerosol radiative forcing. The NASA Langley Research Center airborne High Spectral Resolution Lidar (HSRL-1) has acquired considerable datasets of both aerosol extensive parameters (e.g. aerosol optical depth) and intensive parameters (e.g. aerosol depolarization ratio, lidar ratio) that can be used to infer aerosol type. An aerosol classification methodology has been used extensively to classify HSRL-1 aerosol measurements of different aerosol types including dust, smoke, urban pollution, and marine aerosol. However, atmospheric aerosol is frequently not a single pure type, but instead occurs as a mixture of types, and this mixing affects the optical and radiative properties of the aerosol. Here we present a comprehensive and unified set of rules for characterizing external mixtures using several key aerosol intensive parameters: extinction-to-backscatter ratio (i.e. lidar ratio), backscatter color ratio, and depolarization ratio. Our mixing rules apply not just to the scalar values of aerosol intensive parameters, but to multi-dimensional normal distributions with variance in each measurement dimension. We illustrate the applicability of the mixing rules using examples of HSRL-1 data where mixing occurred between different aerosol types, including advected Saharan dust mixed with the marine boundary layer in the Caribbean Sea and locally generated dust mixed with urban pollution in the Mexico City surroundings. For each of these cases we infer a time-height cross section of mixing ratio along the flight track and we partition aerosol extinction into portions attributed to the two pure types. Since multiple aerosol intensive parameters are measured and included in these calculations, the techniques can also be used for cases without significant depolarization (unlike similar work by earlier researchers), and so a third example of a

  14. Dust Optical Properties Over North Africa and Arabian Peninsula Derived from the AERONET Dataset

    NASA Technical Reports Server (NTRS)

    Kim, D.; Chin, M.; Yu, H.; Eck, T. F.; Sinyuk, A.; Smirnov, A.; Holben, B. N.

    2011-01-01

    Dust optical properties over North Africa and the Arabian Peninsula are extracted from the quality assured multi-year datasets obtained at 14 sites of the Aerosol Robotic Network (AERONET). We select the data with (a) large aerosol optical depth (AOD >= 0.4 at 440 nm) and (b) small Angstrom exponent (A(sub ext)<= 0.2) for retaining high accuracy and reducing interference of non-dust aerosols. The result indicates that the major fraction of high aerosol optical depth days are dominated by dust over these sites even though it varies depending on location and time. We have found that the annual mean and standard deviation of single scattering albedo, asymmetry parameter, real refractive index, and imaginary refractive index for Saharan and Arabian desert dust is 0.944 +/- 0.005, 0.752 +/- 0.014, 1.498 +/- 0.032, and 0.0024 +/- 0.0034 at 550 nm wavelength, respectively. Dust aerosol selected by this method is less absorbing than the previously reported values over these sites. The weaker absorption of dust from this study is consistent with the studies using remote sensing techniques from satellite. These results can help to constrain uncertainties in estimating global dust shortwave radiative forcing.

  15. Global Aerosol Optical Models and Lookup Tables for the New MODIS Aerosol Retrieval over Land

    NASA Technical Reports Server (NTRS)

    Levy, Robert C.; Remer, Loraine A.; Dubovik, Oleg

    2007-01-01

    Since 2000, MODIS has been deriving aerosol properties over land from MODIS observed spectral reflectance, by matching the observed reflectance with that simulated for selected aerosol optical models, aerosol loadings, wavelengths and geometrical conditions (that are contained in a lookup table or 'LUT'). Validation exercises have showed that MODIS tends to under-predict aerosol optical depth (tau) in cases of large tau (tau greater than 1.0), signaling errors in the assumed aerosol optical properties. Using the climatology of almucantur retrievals from the hundreds of global AERONET sunphotometer sites, we found that three spherical-derived models (describing fine-sized dominated aerosol), and one spheroid-derived model (describing coarse-sized dominated aerosol, presumably dust) generally described the range of observed global aerosol properties. The fine dominated models were separated mainly by their single scattering albedo (omega(sub 0)), ranging from non-absorbing aerosol (omega(sub 0) approx. 0.95) in developed urban/industrial regions, to neutrally absorbing aerosol (omega(sub 0) approx.90) in forest fire burning and developing industrial regions, to absorbing aerosol (omega(sub 0) approx. 0.85) in regions of savanna/grassland burning. We determined the dominant model type in each region and season, to create a 1 deg. x 1 deg. grid of assumed aerosol type. We used vector radiative transfer code to create a new LUT, simulating the four aerosol models, in four MODIS channels. Independent AERONET observations of spectral tau agree with the new models, indicating that the new models are suitable for use by the MODIS aerosol retrieval.

  16. Elevated heat pump effects of dust aerosol over Northwestern China during summer

    NASA Astrophysics Data System (ADS)

    Tang, Yaoguo; Han, Yongxiang; Ma, Xiaoyan; Liu, Zhaohuan

    2018-05-01

    The Elevated Heat Pump (EHP) effect demonstrates a significant interaction between the aerosol climatic effect and the monsoon, both are important for climate research. In Northwestern China, the influence of EHP mechanism is still lacking in research. In this study, the EHP effects in Northwestern China are investigated by three sensitivity tests using a WRF-Chem model coupled with the Shao dust emission scheme. Results show that: 1) the anomalous circulation caused by dust aerosols are proved to the existence of EHP effect in Northwestern China; 2) three updrafts over the desert are transported eastward at high altitude and subside in Northeastern China, forming a complete secondary circulation with low-level easterly flow from Badain Jaran and Tengger to Taklimakan; 3) a northeasternerly anomaly flow from Northeastern China can affect the intensity of East Asian summer monsoon (EASM), and increase precipitation in the middle and lower reaches of the Yangtze River and decrease precipitation in Northeastern China. 4) We present a conceptual model of EHP in Northwestern China to provide a better understanding of the climatic effects of dust aerosols.

  17. Dust aerosol properties and radiative forcing observed in spring during 2001-2014 over urban Beijing, China.

    PubMed

    Yu, Xingna; Lü, Rui; Kumar, K Raghavendra; Ma, Jia; Zhang, Qiuju; Jiang, Yilun; Kang, Na; Yang, Suying; Wang, Jing; Li, Mei

    2016-08-01

    The ground-based characteristics (optical and radiative properties) of dust aerosols measured during the springtime between 2001 and 2014 were investigated over urban Beijing, China. The seasonal averaged aerosol optical depth (AOD) during spring of 2001-2014 was about 0.78 at 440 nm. During dust days, higher AOD occurred associated with lower Ångström exponent (AE). The mean AE440-870 in the springtime was about 1.0, indicating dominance of fine particles over the region. The back-trajectory analysis revealed that the dust was transported from the deserts of Inner Mongolia and Mongolia arid regions to Beijing. The aerosol volume size distribution showed a bimodal distribution pattern, with its highest peak observed in coarse mode for all episodes (especially for dust days with increased volume concentration). The single scattering albedo (SSA) increased with wavelength on dust days, indicating the presence of more scattering particles. Furthermore, the complex parts (real and imaginary) of refractive index showed distinct characteristics with lower imaginary values (also scattering) on dust days. The shortwave (SW; 0.2-4.0 μm) and longwave (LW; 4-100 μm) aerosol radiative forcing (ARF) values were computed from the Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART) model both at the top of atmosphere (TOA) and the bottom of atmosphere (BOA) during dust and non-dust (dust free) days, and the corresponding heating rates and forcing efficiencies were also estimated. The SW (LW) ARF, therefore, produced significant cooling (warming) effects at both the TOA and the BOA over Beijing.

  18. Martian Dust Aerosol Size and Shape as Constrained by Phoenix Lander Polarimetry

    NASA Astrophysics Data System (ADS)

    Lemmon, Mark T.; Mason, Emily L.

    2014-11-01

    Dust aerosol morphology is important to dust transport and the radiative heating of the Martian atmosphere. Previous analyses of Mars dust have shown that spherical particles are a bad analog for the dust, in terms of reproducing the distribution of scattered light. Parameterized scattering, based on laboratory observations of scattering by irregular dust particles, has been used for Viking, Pathfinder and Mars Exploration Rover data [Pollack et al., J. Geophys. Res. 100, 1995; Tomasko et al., J. Geophys. Res. 104, 1999; Lemmon et al., Science 306, 2004]. Analytical calculations have shown that cylinders are a better scattering analog than spheres [Wolff et al., J. Geophys. Res. 114, 2009]. Terrestrial studies have shown that a diverse assortment of triaxial ellipsoids is a good analog for dust aerosol [Bi et al., Applied Optics 48, 2009].The Phoenix Lander operated in the Martian arctic for 5 months of 2008, around the northern summer solstice. During the mission atmospheric optical depth was tracked through direct solar imaging by the Surface Stereo Imager (SSI). For solar longitude (Ls) 78-95 and 140-149, small dust storms dominated the weather. Low-dust conditions (optical depths <0.4) dominated during Ls 95-140, with sporadic ice clouds becoming more common after Ls 108. The SSI also obtained occasional cross-sky photometric data through several filters from 440 to 1000 nm and cross-sky polarimetry at 750 nm wavelength. Radiative transfer models of the sky radiance distribution are consistent with dust aerosols in the same 1.3-1.6 micron range reported for models of observations from previous missions. Cylinders, triaxial ellipsoids, and the parametric model can fit sky radiances; spheres cannot. The observed linear polarization, which reached 4-5% and had a similar angular distribution to Rayleigh polarization, is similar to the triaxial ellipsoid model, but not spheres or cylinders. An extension to the parametric model using 7-10% Rayleigh scattering mixed

  19. Refractive Index and Absorption Attribution of Highly Absorbing Brown Carbon Aerosols from an Urban Indian City-Kanpur.

    PubMed

    Shamjad, P M; Tripathi, S N; Thamban, Navaneeth M; Vreeland, Heidi

    2016-11-24

    Atmospheric aerosols influence Earth's radiative balance, having both warming and cooling effects. Though many aerosols reflect radiation, carbonaceous aerosols such as black carbon and certain organic carbon species known as brown carbon have the potential to warm the atmosphere by absorbing light. Black carbon absorbs light over the entire solar spectrum whereas brown carbon absorbs near-UV wavelengths and, to a lesser extent, visible light. In developing countries, such as India, where combustion sources are prolific, the influence of brown carbon on absorption may be significant. In order to better characterize brown carbon, we present experimental and modeled absorption properties of submicron aerosols measured in an urban Indian city (Kanpur). Brown carbon here is found to be fivefold more absorbing at 365 nm wavelength compared to previous studies. Results suggest ~30% of total absorption in Kanpur is attributed to brown carbon, with primary organic aerosols contributing more than secondary organics. We report the spectral brown carbon refractive indices along with an experimentally constrained estimate of the influence of aerosol mixing state on absorption. We conclude that brown carbon in Kanpur is highly absorbing in nature and that the mixing state plays an important role in light absorption from volatile species.

  20. Refractive Index and Absorption Attribution of Highly Absorbing Brown Carbon Aerosols from an Urban Indian City-Kanpur

    PubMed Central

    Shamjad, P. M.; Tripathi, S. N.; Thamban, Navaneeth M.; Vreeland, Heidi

    2016-01-01

    Atmospheric aerosols influence Earth’s radiative balance, having both warming and cooling effects. Though many aerosols reflect radiation, carbonaceous aerosols such as black carbon and certain organic carbon species known as brown carbon have the potential to warm the atmosphere by absorbing light. Black carbon absorbs light over the entire solar spectrum whereas brown carbon absorbs near-UV wavelengths and, to a lesser extent, visible light. In developing countries, such as India, where combustion sources are prolific, the influence of brown carbon on absorption may be significant. In order to better characterize brown carbon, we present experimental and modeled absorption properties of submicron aerosols measured in an urban Indian city (Kanpur). Brown carbon here is found to be fivefold more absorbing at 365 nm wavelength compared to previous studies. Results suggest ~30% of total absorption in Kanpur is attributed to brown carbon, with primary organic aerosols contributing more than secondary organics. We report the spectral brown carbon refractive indices along with an experimentally constrained estimate of the influence of aerosol mixing state on absorption. We conclude that brown carbon in Kanpur is highly absorbing in nature and that the mixing state plays an important role in light absorption from volatile species. PMID:27883083

  1. Dust aerosols above the south polar cap of Mars as seen by OMEGA

    NASA Astrophysics Data System (ADS)

    Vincendon, M.; Langevin, Y.; Poulet, F.; Bibring, J.-P.; Gondet, B.; Jouglet, D.; Omega Team

    2008-08-01

    The time evolution of atmospheric dust at high southern latitudes on Mars has been determined using observations of the south seasonal cap acquired in the near infrared (1-2.65 μm) by OMEGA/Mars Express in 2005. Observations at different solar zenith angles and one EPF sequence demonstrate that the reflectance in the 2.64 μm saturated absorption band of the surface CO 2 ice is mainly due to the light scattered by aerosols above most places of the seasonal cap. We have mapped the total optical depth of dust aerosols in the near-IR above the south seasonal cap of Mars from mid-spring to early summer with a time resolution ranging from one day to one week and a spatial resolution of a few kilometers. The optical depth above the south perennial cap is determined on a longer time range covering southern spring and summer. A constant set of optical properties of dust aerosols is consistent with OMEGA observations during the analyzed period. Strong variations of the optical depth are observed over small horizontal and temporal scales, corresponding in part to moving dust clouds. The late summer peak in dust opacity observed by Opportunity in 2005 propagated to the south pole contrarily to that observed in mid spring. This may be linked to evidence for dust scavenging by water ice-rich clouds circulating at high southern latitudes at this season.

  2. Longwave Radiative Forcing of Saharan Dust Aerosols Estimated from MODIS, MISR and CERES Observations on Terra

    NASA Technical Reports Server (NTRS)

    Zhang, Jiang-Long; Christopher, Sundar A.

    2003-01-01

    Using observations from the Multi-angle Imaging Spectroradiometer (MISR), the Moderate Resolution Imaging Spectroradiometer (MODIS), and the Clouds and the Earth's Radiant Energy System (CERES) instruments onboard the Terra satellite; we present a new technique for studying longwave (LW) radiative forcing of dust aerosols over the Saharan desert for cloud-free conditions. The monthly-mean LW forcing for September 2000 is 7 W/sq m and the LW forcing efficiency' (LW(sub eff)) is 15 W/sq m. Using radiative transfer calculations, we also show that the vertical distribution of aerosols and water vapor are critical to the understanding of dust aerosol forcing. Using well calibrated, spatially and temporally collocated data sets, we have combined the strengths of three sensors from the same satellite to quantify the LW radiative forcing, and show that dust aerosols have a "warming" effect over the Saharan desert that will counteract the shortwave "cooling effect" of aerosols.

  3. Seventeen-year systematic measurements of dust aerosol optical properties using the eole ntua lidar system (2000-2016)

    NASA Astrophysics Data System (ADS)

    Soupiona, Ourania; Mylonaki, Maria; Papayannis, Alexandros; Argyrouli, Athina; Kokkalis, Panayotis; Tsaknakis, Georgios

    2018-04-01

    A comprehensive analysis of the seasonal variability of the optical properties of Saharan dust aerosols over Athens, Greece, is presented for a 17-year time period (2000-2016), as derived from multi-wavelength Raman lidar measurements (57 dust events with more than 80 hours of measurements). The profiles of the derived aerosol optical properties (aerosol backscatter and extinction coefficients, lidar ratio and aerosol Ångström exponent) at 355 nm are presented. For these dust events we found a mean value of the lidar ratio of 52±13 sr at 355 nm and of 58±8 sr (not shown) at 532 nm (2-4 km a.s.l. height). For our statistical analysis, presented here, we used monthly-mean values and time periods under cloud-free conditions. The number of dust events was greatest in late spring, summer, and early autumn periods. In this paper we also present a selected case study (04 April 2016) of desert dust long-range transport from the Saharan desert.

  4. Studies on aerosols. I. Reduction of dust deposition in lungs of rabbits by aqueous aerosols

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dautrebande, L.; Highman, B.; Alford, W.C.

    1948-01-01

    Rabbits were exposed to air containing 0.01 to 0.04 mg/liter zinc silicate dust with a mean diameter of 0.9 ..mu..m. Irregular breathing with some cyanosis after 2 hr was observed. Pulmonary changes after 4.5 to 5 hr included bronchitis, patchy atelectasis, emphysema, interstitial pneumonitis (thickening of septa, moderate congestion, infiltration of mononuclear cells and polymorphonuclear leukocytes). After 1, 7, or 14 days recovery there were no or only slight pulmonary problems. There was localization of particles at surfaces facing, deflecting or slowing air currents, particularly near pleura and hilus and less in central portion of lobes. Rabbits exposed to abovemore » dust plus aqueous wetting agent aerosol averaging 0.5 ..mu..m in diameter showed no cyanosis or marked respiratory difficulty. Rabbits showed less of above pulmonary changes and lesser amount of dust in lungs, particularly in alveoli and alveolar ducts. Most particles were cleared in 1 day in both groups, especially aerosol group, and essentially were all gone after 7 days. Differences were primarily due to coating of particles with liquid (increased size) and aggregation.« less

  5. Impacts of Snow Darkening by Absorbing Aerosols on Eurasian Climate

    NASA Technical Reports Server (NTRS)

    Kim, Kyu-Myong; Lau, William K M.; Yasunari, Teppei J.; Kim, Maeng-Ki; Koster, Randal D.

    2016-01-01

    The deposition of absorbing aerosols on snow surfaces reduces snow-albedo and allows snowpack to absorb more sunlight. This so-called snow darkening effect (SDE) accelerates snow melting and leads to surface warming in spring. To examine the impact of SDE on weather and climate during late spring and early summer, two sets of NASA GEOS-5 model simulations with and without SDE are conducted. Results show that SDE-induced surface heating is particularly pronounced in Eurasian regions where significant depositions of dust transported from the North African deserts, and black carbon from biomass burning from Asia and Europe occur. In these regions, the surface heating due to SDE increases surface skin temperature by 3-6 degrees Kelvin near the snowline in spring. Surface energy budget analysis indicates that SDE-induced excess heating is associated with a large increase in surface evaporation, subsequently leading to a significant reduction in soil moisture, and increased risks of drought and heat waves in late spring to early summer. Overall, we find that rainfall deficit combined with SDE-induced dry soil in spring provide favorable condition for summertime heat waves over large regions of Eurasia. Increased frequency of summer heat waves with SDE and the region of maximum increase in heat-wave frequency are found along the snow line, providing evidence that early snowmelt by SDE may increase the risks of extreme summer heat wave. Our results suggest that climate models that do not include SDE may significantly underestimate the effect of global warming over extra-tropical continental regions.

  6. Dust Aerosol Particle Size at the Mars Science Laboratory Landing Site

    NASA Astrophysics Data System (ADS)

    Vicente-Retortillo, Alvaro; Martínez, Germán; Renno, Nilton; Lemmon, Mark; de la Torre-Juárez, Manuel

    2017-04-01

    We have developed a new methodology to retrieve dust aerosol particle size from Mars Science Laboratory (MSL) observations [1]. We use photodiode output currents measured by the Rover Environmental Monitoring Station (REMS) UV sensor (UVS), ancillary data records (ADR) containing the geometry of the rover and the Sun, and values of the atmospheric opacity retrieved from Mastcam measurements. In particular, we analyze REMS UVS measurements when the Sun is blocked by the masthead and the mast of the rover since the behavior of the output currents during these shadow events depends on the dust phase function, which depends on particle size. The retrieved dust effective radii show a significant seasonal variability, ranging from 0.6 μm during the low opacity season (Ls = 60° - 140°) to 2 μm during the high opacity season (Ls = 180° - 360°). The relationship between atmospheric opacity and dust particle size indicates that dust-lifting events originate at various distances from Gale Crater. The external origin of high dust content events is consistent with the strong and persistent northerly and northwesterly winds at Gale Crater during the perihelion season centered around Ls = 270° [2]. From an interannual perspective, the general behavior of the particle size evolution in MY 31-32 is similar to that in MY 32-33, although some differences are noted. During the low opacity season (Ls = 60° - 140°), the retrieved dust effective radii in MY 33 are significantly lower than in MY 32. A larger contribution of water ice clouds to the total atmospheric opacity during the aphelion season of MY 33 can partially explain such a departure. Differences during the perihelion season are caused by interannual variability of enhanced opacity events. The determination of dust aerosol particle size is important to improve the accuracy of models in simulating the UV environment at the surface [3] and in predicting heating rates, which affect the atmospheric thermal and dynamical

  7. Asian dust aerosol: Optical effect on satellite ocean color signal and a scheme of its correction

    NASA Astrophysics Data System (ADS)

    Fukushima, H.; Toratani, M.

    1997-07-01

    The paper first exhibits the influence of the Asian dust aerosol (KOSA) on a coastal zone color scanner (CZCS) image which records erroneously low or negative satellite-derived water-leaving radiance especially in a shorter wavelength region. This suggests the presence of spectrally dependent absorption which was disregarded in the past atmospheric correction algorithms. On the basis of the analysis of the scene, a semiempirical optical model of the Asian dust aerosol that relates aerosol single scattering albedo (ωA) to the spectral ratio of aerosol optical thickness between 550 nm and 670 nm is developed. Then, as a modification to a standard CZCS atmospheric correction algorithm (NASA standard algorithm), a scheme which estimates pixel-wise aerosol optical thickness, and in turn ωA, is proposed. The assumption of constant normalized water-leaving radiance at 550 nm is adopted together with a model of aerosol scattering phase function. The scheme is combined to the standard algorithm, performing atmospheric correction just the same as the standard version with a fixed Angstrom coefficient except in the case where the presence of Asian dust aerosol is detected by the lowered satellite-derived Angstrom exponent. Some of the model parameter values are determined so that the scheme does not produce any spatial discontinuity with the standard scheme. The algorithm was tested against the Japanese Asian dust CZCS scene with parameter values of the spectral dependency of ωA, first statistically determined and second optimized for selected pixels. Analysis suggests that the parameter values depend on the assumed Angstrom coefficient for standard algorithm, at the same time defining the spatial extent of the area to apply the Asian dust scheme. The algorithm was also tested for a Saharan dust scene, showing the relevance of the scheme but with different parameter setting. Finally, the algorithm was applied to a data set of 25 CZCS scenes to produce a monthly composite

  8. Intensification of North American Megadroughts through Surface and Dust Aerosol Forcing

    NASA Technical Reports Server (NTRS)

    Cook, Benjamin I.; Seager, Richard; Miller, Ron L.; Mason, Joseph A

    2013-01-01

    Tree-ring-based reconstructions of the Palmer drought severity index (PDSI) indicate that, during the Medieval Climate Anomaly (MCA), the central plains of North America experienced recurrent periods of drought spanning decades or longer. These megadroughts had exceptional persistence compared to more recent events, but the causes remain uncertain. The authors conducted a suite of general circulation model experiments to test the impact of sea surface temperature (SST) and land surface forcing on the MCA megadroughts over the central plains. The land surface forcing is represented as a set of dune mobilization boundary conditions, derived from available geomorphological evidence and modeled as increased bare soil area and a dust aerosol source (32deg-44degN, 105deg-95degW). In the experiments, cold tropical Pacific SST forcing suppresses precipitation over the central plains but cannot reproduce the overall drying or persistence seen in the PDSI reconstruction. Droughts in the scenario with dust aerosols, however, are amplified and have significantly longer persistence than in other model experiments, more closely matching the reconstructed PDSI. This additional drying occurs because the dust increases the shortwave planetary albedo, reducing energy inputs to the surface and boundary layer. The energy deficit increases atmospheric stability, inhibiting convection and reducing cloud cover and precipitation over the central plains. Results from this study provide the first model-based evidence that dust aerosol forcing and land surface changes could have contributed to the intensity and persistence of the central plains megadroughts, although uncertainties remain in the formulation of the boundary conditions and the future importance of these feedbacks.

  9. Long-range-transported Saharan dust in the Caribbean - an electron microscopy perspective of aerosol composition and modification

    NASA Astrophysics Data System (ADS)

    Kandler, Konrad; Hartmann, Markus; Ebert, Martin; Weinbruch, Stephan; Weinzierl, Bernadett; Walser, Adrian; Sauer, Daniel; Wadinga Fomba, Khanneh

    2015-04-01

    From June to July in 2013, the Saharan Aerosol Long-range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE) was performed in the Caribbean. Airborne aerosol sampling was performed onboard the DLR Falcon aircraft in altitudes between 300 m and 5500 m. Ground-based samples were collected at Ragged Point (Barbados, 13.165 °N, 59.432 °W) and at the Cape Verde Atmospheric Observatory (Sao Vicente, 16.864 °N, 24.868 °W). Different types of impactors and sedimentation samplers were used to collect particles between 0.1 µm and 4 µm (airborne) and between 0.1 µm and 100 µm (ground-based). Particles were analyzed by scanning electron microscopy with attached energy-dispersive X-ray analysis, yielding information on particle size, particle shape and chemical composition for elements heavier than nitrogen. A particle size correction was applied to the chemical data to yield better quantification. A total of approximately 100,000 particles were analyzed. For particles larger than 0.7 µm, the aerosol in the Caribbean during the campaign was a mixture of mineral dust, sea-salt at different aging states, and sulfate. Inside the Saharan dust plume - outside the marine boundary layer (MBL) - the aerosol is absolutely dominated by mineral dust. Inside the upper MBL, sea-salt exists as minor component in the aerosol for particles smaller than 2 µm in diameter, larger ones are practically dust only. When crossing the Soufriere Hills volcano plume with the aircraft, an extremely high abundance of small sulfate particles could be observed. At Ragged Point, in contrast to the airborne measurements, aerosol is frequently dominated by sea-salt particles. Dust relative abundance at Ragged Point has a maximum between 5 µm and 10 µm particles diameter; at larger sizes, sea-salt again prevails due to the sea-spray influence. A significant number of dust particles larger than 20 µm was encountered. The dust component in the Caribbean - airborne as well as ground

  10. Characterization of Optical Properties of Desert Dust and Other Aerosols Using Postive Matrix Factorization

    NASA Astrophysics Data System (ADS)

    Lihavainen, H.; Alghamdi, M.; Hyvärinen, A.; Hussein, T.; Neitola, K.; Khoder, M.; Abdelmaksoud, A. S.; Al-Jeelani, H.; Shabbaj, I. I.; Almehmadi, F. M.

    2017-12-01

    To derive the comprehensive aerosol in situ characteristics at a rural background area in Saudi Arabia, an aerosol measurements station was established to Hada Al Sham, 60 km east from the Red Sea and the city of Jeddah. The present sturdy describes the observational data from February 2013 to February 2015 of scattering and absorption coefficients, Ångström exponents and single scattering albedo over the measurement period. As expected, the scattering coefficient was dominated by large desert dust particles with low Ångström scattering exponent. Especially from February to June the Ångström scattering exponent was clearly lower and scattering coefficients higher than total averages because of the dust outbreak season. Aerosol optical properties had clear diurnal cycle. The lowest scattering and absorption coefficients and aerosol optical depths were observed around noon. The observed diurnal variation is caused by wind direction and speed, during night time very calm easterly winds are dominating whereas during daytime the stronger westerly winds are dominating (sea breeze). Positive Matrix Factorization mathematical tool was applied to the scattering and absorption coefficients and PM2.5 and coarse mode (PM10- PM2.5) mass concentrations to characterise aerosols from different sources. Analysis revealed three clearly different types of sources, anthropogenic, BC source and desert dust. These factors have clearly different seasonal and diurnal variation. The contribution of desert dust factor was dominating from February to May, whereas the contribution of anthropogenic factor is quite steady over the whole year. We estimated the mass absorption and scattering efficiencies for the factors and they agreed well with earlier observations. Hence, this method could be used to distinguish aerosol source characteristics, at least in fairly simple cases.

  11. Measurement-based estimates of direct radiative effects of absorbing aerosols above clouds

    NASA Astrophysics Data System (ADS)

    Feng, Nan; Christopher, Sundar A.

    2015-07-01

    The elevated layers of absorbing smoke aerosols from western African (e.g., Gabon and Congo) biomass burning activities have been frequently observed above low-level stratocumulus clouds off the African coast, which presents an excellent natural laboratory for studying the effects of aerosols above clouds (AAC) on regional energy balance in tropical and subtropical environments. Using spatially and temporally collocated Moderate Resolution Imaging Spectroradiometer, Ozone Monitoring Instrument (OMI), and Clouds and the Earth's Radiant Energy System data sets, the top-of-atmosphere shortwave aerosol direct shortwave radiative effects (ARE) of absorbing aerosols above low-level water clouds in the southeast Atlantic Ocean was examined in this study. The regional averaged instantaneous ARE has been estimated to be 36.7 ± 20.5 Wm-2 (regional mean ± standard deviation) along with a mean positive OMI Aerosol Index at 1.3 in August 2006 based on multisensors measurements. The highest magnitude of instantaneous ARE can even reach 138.2 Wm-2. We assess that the 660 nm cloud optical depth (COD) values of 8-12 is the critical value above (below) which aerosol absorption (scattering) effect dominates and further produces positive (negative) ARE values. The results further show that ARE values are more sensitive to aerosols above lower COD values than cases for higher COD values. This is among the first studies to provide quantitative estimates of shortwave ARE due to AAC events from an observational perspective.

  12. A New Method Using Single-Particle Mass Spectrometry Data to Distinguish Mineral Dust and Biological Aerosols

    NASA Astrophysics Data System (ADS)

    Al-Mashat, H.; Kristensen, L.; Sultana, C. M.; Prather, K. A.

    2016-12-01

    The ability to distinguish types of particles present within a cloud is important for determining accurate inputs to climate models. The chemical composition of particles within cloud liquid droplets and ice crystals can have a significant impact on the timing, location, and amount of precipitation that falls. Precipitation efficiency is increased by the presence of ice crystals in clouds, and both mineral dust and biological aerosols have been shown to be effective ice nucleating particles (INPs) in the atmosphere. A current challenge in aerosol science is distinguishing mineral dust and biological material in the analysis of real-time, ambient, single-particle mass spectral data. Single-particle mass spectrometers are capable of measuring the size-resolved chemical composition of individual atmospheric particles. However, there is no consistent analytical method for distinguishing dust and biological aerosols. Sampling and characterization of control samples (i.e. of known identity) of mineral dust and bacteria were performed by the Aerosol Time-of-Flight Mass Spectrometer (ATOFMS) as part of the Fifth Ice Nucleation (FIN01) Workshop at the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) facility in Karlsruhe, Germany. Using data collected by the ATOFMS of control samples, a new metric has been developed to classify single particles as dust or biological independent of spectral cluster analysis. This method, involving the use of a ratio of mass spectral peak areas for organic nitrogen and silicates, is easily reproducible and does not rely on extensive knowledge of particle chemistry or the ionization characteristics of mass spectrometers. This represents a step toward rapidly distinguishing particle types responsible for ice nucleation activity during real-time sampling in clouds. The ability to distinguish types of particles present within a cloud is important for determining accurate inputs to climate models. The chemical composition of particles

  13. Possible influence of dust on hurricane genesis

    NASA Astrophysics Data System (ADS)

    Bretl, Sebastian; Reutter, Philipp; Raible, Christoph C.; Ferrachat, Sylvaine; Lohmann, Ulrike

    2014-05-01

    Tropical Cyclones (TCs) belong to the most extreme events in nature. In the past decade, the possible impact of dust on Atlantic hurricanes receives growing interest. As mineral dust is able to absorb incoming solar radiation and therefore warm the surrounding air, the presence of dust can lead to a reduction of sea surface temperature (SST) and an increase in atmospheric stability. Furthermore, resulting baroclinic effects and the dry Saharan easterly jet lead to an enhanced vertical shear of the horizontal winds. SST, stability, moisture and vertical wind shear are known to potentially impact hurricane activity. But how Saharan dust influences these prerequisites for hurricane formation is not yet clear. Some dynamical mechanisms induced by the SAL might even strengthen hurricanes. An adequate framework for investigating the possible impact of dust on hurricanes is comparing high resolution simulations (~0.5°x0.5°, 31 vertical levels) with and without radiatively active dust aerosols. To accomplish this task, we are using the general circulation model ECHAM6 coupled to a modified version of the aerosol model HAM, ECHAM6-HAM-Dust. Instead of the five aerosol species HAM normally contains, the modified version takes only insoluble dust into account, but modifies the scavenging parameters in order to have a similar lifetime of dust as in the full ECHAM6-HAM. All remaining aerosols are prescribed. To evaluate the effects of dust on hurricanes, a TC detection and tracking method is applied on the results. ECHAM6-HAM-Dust was used in two configurations, one with radiatively active dust aerosols and one with dust being not radiatively active. For both set-ups, 10 Monte-Carlo simulations of the year 2005 were performed. A statistical method which identifies controlling parameters of hurricane genesis was applied on North Atlantic developing and non-developing disturbances in all simulations, comparing storms in the two sets of simulations. Hereby, dust can be assigned

  14. Impact of Saharan dust on North Atlantic marine stratocumulus clouds: importance of the semidirect effect

    NASA Astrophysics Data System (ADS)

    Amiri-Farahani, Anahita; Allen, Robert J.; Neubauer, David; Lohmann, Ulrike

    2017-05-01

    One component of aerosol-cloud interactions (ACI) involves dust and marine stratocumulus clouds (MSc). Few observational studies have focused on dust-MSc interactions, and thus this effect remains poorly quantified. We use observations from multiple sensors in the NASA A-Train satellite constellation from 2004 to 2012 to obtain estimates of the aerosol-cloud radiative effect, including its uncertainty, of dust aerosol influencing Atlantic MSc off the coast of northern Africa between 45° W and 15° E and between 0 and 35° N. To calculate the aerosol-cloud radiative effect, we use two methods following Quaas et al. (2008) (Method 1) and Chen et al. (2014) (Method 2). These two methods yield similar results of -1.5 ± 1.4 and -1.5 ± 1.6 W m-2, respectively, for the annual mean aerosol-cloud radiative effect. Thus, Saharan dust modifies MSc in a way that acts to cool the planet. There is a strong seasonal variation, with the aerosol-cloud radiative effect switching from significantly negative during the boreal summer to weakly positive during boreal winter. Method 1 (Method 2) yields -3.8 ± 2.5 (-4.3 ± 4.1) during summer and 1 ± 2.9 (0.6 ± 1) W m-2 during winter. In Method 1, the aerosol-cloud radiative effect can be decomposed into two terms, one representing the first aerosol indirect effect and the second representing the combination of the second aerosol indirect effect and the semidirect effect (i.e., changes in liquid water path and cloud fraction in response to changes in absorbing aerosols and local heating). The first aerosol indirect effect is relatively small, varying from -0.7 ± 0.6 in summer to 0.1 ± 0.5 W m-2 in winter. The second term, however, dominates the overall radiative effect, varying from -3.2 ± 2.5 in summer to 0.9 ± 2.9 W m-2 during winter. Studies show that the semidirect effect can result in a negative (i.e., absorbing aerosol lies above low clouds like MSc) or positive (i.e., absorbing aerosol lies within low clouds) aerosol

  15. Predicting the Mineral Composition of Dust Aerosols. Part 1; Representing Key Processes

    NASA Technical Reports Server (NTRS)

    Perlwitz, J. P.; Garcia-Pando, C. Perez; Miller, R. L.

    2015-01-01

    Soil dust aerosols created by wind erosion are typically assigned globally uniform physical and chemical properties within Earth system models, despite known regional variations in the mineral content of the parent soil. Mineral composition of the aerosol particles is important to their interaction with climate, including shortwave absorption and radiative forcing, nucleation of cloud droplets and ice crystals, heterogeneous formation of sulfates and nitrates, and atmospheric processing of iron into bioavailable forms that increase the productivity of marine phytoplankton. Here, aerosol mineral composition is derived by extending a method that provides the composition of a wet-sieved soil. The extension accounts for measurements showing significant differences between the mineral fractions of the wetsieved soil and the emitted aerosol concentration. For example, some phyllosilicate aerosols are more prevalent at silt sizes, even though they are nearly absent at these diameters in a soil whose aggregates are dispersed by wet sieving. We calculate the emitted mass of each mineral with respect to size by accounting for the disintegration of soil aggregates during wet sieving. These aggregates are emitted during mobilization and fragmentation of the original undispersed soil that is subject to wind erosion. The emitted aggregates are carried far downwind from their parent soil. The soil mineral fractions used to calculate the aggregates also include larger particles that are suspended only in the vicinity of the source. We calculate the emitted size distribution of these particles using a normalized distribution derived from aerosol measurements. In addition, a method is proposed for mixing minerals with small impurities composed of iron oxides. These mixtures are important for transporting iron far from the dust source, because pure iron oxides are more dense and vulnerable to gravitational removal than most minerals comprising dust aerosols. A limited comparison to

  16. Predicting the mineral composition of dust aerosols - Part 1: Representing key processes

    NASA Astrophysics Data System (ADS)

    Perlwitz, J. P.; Pérez García-Pando, C.; Miller, R. L.

    2015-10-01

    Soil dust aerosols created by wind erosion are typically assigned globally uniform physical and chemical properties within Earth system models, despite known regional variations in the mineral content of the parent soil. Mineral composition of the aerosol particles is important to their interaction with climate, including shortwave absorption and radiative forcing, nucleation of cloud droplets and ice crystals, heterogeneous formation of sulfates and nitrates, and atmospheric processing of iron into bioavailable forms that increase the productivity of marine phytoplankton. Here, aerosol mineral composition is derived by extending a method that provides the composition of a wet-sieved soil. The extension accounts for measurements showing significant differences between the mineral fractions of the wet-sieved soil and the emitted aerosol concentration. For example, some phyllosilicate aerosols are more prevalent at silt sizes, even though they are nearly absent at these diameters in a soil whose aggregates are dispersed by wet sieving. We calculate the emitted mass of each mineral with respect to size by accounting for the disintegration of soil aggregates during wet sieving. These aggregates are emitted during mobilization and fragmentation of the original undispersed soil that is subject to wind erosion. The emitted aggregates are carried far downwind from their parent soil. The soil mineral fractions used to calculate the aggregates also include larger particles that are suspended only in the vicinity of the source. We calculate the emitted size distribution of these particles using a normalized distribution derived from aerosol measurements. In addition, a method is proposed for mixing minerals with small impurities composed of iron oxides. These mixtures are important for transporting iron far from the dust source, because pure iron oxides are more dense and vulnerable to gravitational removal than most minerals comprising dust aerosols. A limited comparison to

  17. Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing During Boreal Spring

    NASA Technical Reports Server (NTRS)

    Kim, Maeng-Ki; Lau, K. M.; Chin, Mian; Kim, Kyu-Myong; Sud, Y. C.; Walker, Greg K.

    2005-01-01

    The direct effects of aerosols on global and regional climate during boreal spring are investigated based on simulations using the NASA Global Modeling and Assimilation Office (GMAO) finite-volume general circulation model (fvGCM) with Microphyics of clouds in Relaxed Arakawa Schubert Scheme (McRAS). The aerosol loading are prescribed from three-dimensional monthly distribution of tropospheric aerosols viz., sulfate, black carbon, organic carbon, soil dust, and sea salt from output of the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The aerosol extinction coefficient, single scattering albedo, and asymmetric factor are computed as wavelength-dependent radiative forcing in the radiative transfer scheme of the fvGCM, and as a function of the aerosol loading and ambient relative humidity. We find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excites a planetary scale teleconnection pattern in sea level pressure, temperature and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, i.e., South Asia, East Asia, and northern and western Africa. Additionally, atmospheric heating is found in regions with large loading of dust (over Northern Africa, and Middle East), and black carbon (over South-East Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east-west dipole anomaly with strong cooling over the Caspian Sea, and warming over central and northeastern Asia, where aerosol concentration are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes

  18. MPL Guwahati and extraction of aerosol and dust features

    NASA Astrophysics Data System (ADS)

    Devi, M.; Baishy, R.; Barbara, A.

    Aerosols emitted directly from natural and anthropogenic sources are responsible for bringing changes in atmospheric conditions and in modifying physical and dynamical processes therein. With the aim to correlate such changes in atmospheric environments with aerosols, a MPL Lidar has been put into operation at Gauhati University a subtropical station, where atmospheric variabilities are subjected to the influence of its complex local topography and man made system inhomogenities. The Lidar that is in operation at Gauhati University since January 2001, has been developed in collaboration with Chiba University, Japan. This portable instrument consists of a low power (>20 μ Jule) 10 ns pulse laser at 532 nm with PRF varying from 1 to 5 KHz. The receiver consists of a 0.2 m aperture case grain telescope with 1nm filter and the PMT working in photon counting mode. The signal acquisition is done in LabVIEW environment and processing is made through a user-friendlyn software also in LabVIEW environment developed by this group. The aerosol and dust signatures received through routine sounding are analyzed for extinction and backscattered cross section parameters and attempts are made for evaluating significant features in backscattered signal from dust particles which are well detected in the lidar echogram during early spring. The paper also discusses the techniques for evaluation of system constant "C" before presenting cross section parameters. The approach is through horizontal probing of the atmosphere and assuming same type of aerosol population over a defined (near surface) altitude. The "C" value so obtained, comes close to the figure calculated from relation,

  19. Dust, Pollution, and Biomass Burning Aerosols in Asian Pacific: A Column Surface/Satellite Perspective

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Lau, William K. M. (Technical Monitor)

    2002-01-01

    Many recent field experiments are designed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern/southeastern Asia and along the rim of the western Pacific. For example, the phase-I of ACE-Asia was conducted from March-May 2001 in the vicinity of the Gobi desert, East Coast of China, Yellow Sea, Korea, and Japan, along the pathway of Kosa (severe events that blanket East Asia with yellow desert dust, peaked in the Spring season). Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Springtime is also the peak season for biomass burning in southeastern Asia. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian aerosols is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia we have measured continuously aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over homogeneous areas from surface. The inclusion of flux measurements permits the determination of aerosol radiative flux in addition to measurements of loading and optical depth. At the time of the Terra/MODIS (Moderate Resolution Imaging Spectroradiometer), SeaWiFS (Sea-viewing Wide Field-of-view Sensor), TOMS (Total Ozone Mapping Spectrometer) and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. A column satellite-surface perspective of Asian aerosols will be presented

  20. Tropical Atlantic Dust and Smoke Aerosol Variabilities Related to the Madden-Julian Oscillation in MODIS and MISR Observations

    NASA Technical Reports Server (NTRS)

    Guo, Yanjuan; Tian, Baijun; Kahn, Ralph A.; Kalashnikova, Olga; Wong, Sun; Waliser, Duane E.

    2012-01-01

    In this study, MODIS fine mode fraction and MISR non-spherical fraction are 2used to derive dust and smoke AOT components (tau(sub dust) and tau(sub smoke)) over the tropical Atlantic, and their variabilities related to the Madden-Julian Oscillation (MJO) are then investigated. Both MODIS and MISR show a very similar dust and smoke winter climatology. tau(sub dust) is found to be the dominant aerosol component over the tropical Atlantic while tau(sub smoke) is significantly smaller than tau(sub dust). The daily MODIS and MISR tau(sub dust) are overall highly correlated, with the correlation coefficients typically about 0.7 over the North Atlantic. The consistency between the MODIS and MISR dust and smoke aerosol climatology and daily variations give us confidence to use these two data sets to investigate their relative contributions to the total AOT variation associated with the MJO. However, unlike the MISR dust discrimination, which is based on particle shape retrievals, the smoke discrimination is less certain, based on assumed partitioning of maritime aerosol for both MISR and MODIS. The temporal evolution and spatial patterns of the tau(sub dust) anomalies associated with the MJO are consistent between MODIS and MISR. The tau(sub dust) anomalies are very similar to those of tau anomalies, and are of comparable magnitude. In contrast, the MJO-related tau(sub smoke) anomalies are rather small, and the tau(sub mar) anomalies are negligible. The consistency between the MODIS and MISR results suggests that dust aerosol is the dominant component on the intra-seasonal time scale over the tropical Atlantic Ocean.

  1. Investigating cloud absorption effects: Global absorption properties of black carbon, tar balls, and soil dust in clouds and aerosols

    NASA Astrophysics Data System (ADS)

    Jacobson, Mark Z.

    2012-03-01

    This study examines modeled properties of black carbon (BC), tar ball (TB), and soil dust (SD) absorption within clouds and aerosols to understand better Cloud Absorption Effects I and II, which are defined as the effects on cloud heating of absorbing inclusions in hydrometeor particles and of absorbing aerosol particles interstitially between hydrometeor particles at their actual relative humidity (RH), respectively. The globally and annually averaged modeled 550 nm aerosol mass absorption coefficient (AMAC) of externally mixed BC was 6.72 (6.3-7.3) m2/g, within the laboratory range (6.3-8.7 m2/g). The global AMAC of internally mixed (IM) BC was 16.2 (13.9-18.2) m2/g, less than the measured maximum at 100% RH (23 m2/g). The resulting AMAC amplification factor due to internal mixing was 2.41 (2-2.9), with highest values in high RH regions. The global 650 nm hydrometeor mass absorption coefficient (HMAC) due to BC inclusions was 17.7 (10.6-19) m2/g, ˜9.3% higher than that of the IM-AMAC. The 650 nm HMACs of TBs and SD were half and 1/190th, respectively, that of BC. Modeled aerosol absorption optical depths were consistent with data. In column tests, BC inclusions in low and mid clouds (CAE I) gave column-integrated BC heating rates ˜200% and 235%, respectively, those of interstitial BC at the actual cloud RH (CAE II), which itself gave heating rates ˜120% and ˜130%, respectively, those of interstitial BC at the clear-sky RH. Globally, cloud optical depth increased then decreased with increasing aerosol optical depth, consistent with boomerang curves from satellite studies. Thus, CAEs, which are largely ignored, heat clouds significantly.

  2. Sunlight Transmission through Desert Dust and Marine Aerosols: Diffuse Light Corrections to Sun Photometry and Pyrheliometry

    NASA Technical Reports Server (NTRS)

    Russell, P. B.; Livingston, J. M.; Dubovik, O.; Ramirez, S. A.; Wang, J.; Redemann, J.; Schmid, B.; Box, M.; Holben, B. N.

    2003-01-01

    Desert dust and marine aerosols are receiving increased scientific attention because of their prevalence on intercontinental scales and their potentially large effects on Earth radiation and climate, as well as on other aerosols, clouds, and precipitation. The relatively large size of desert dust and marine aerosols produces scattering phase functions that are strongly forward- peaked. Hence, Sun photometry and pyrheliometry of these aerosols are more subject to diffuse-light errors than is the case for smaller aerosols. Here we quantify these diffuse-light effects for common Sun photometer and pyrheliometer fields of view (FOV), using a data base on dust and marine aerosols derived from (1) AERONET measurements of sky radiance and solar beam transmission and (2) in situ measurements of aerosol layer size distribution and chemical composition. Accounting for particle non-sphericity is important when deriving dust size distribution from both AERONET and in situ aerodynamic measurements. We express our results in terms of correction factors that can be applied to Sun photometer and pyrheliometer measurements of aerosol optical depth (AOD). We find that the corrections are negligible (less than approximately 1% of AOD) for Sun photometers with narrow FOV (half-angle eta less than degree), but that they can be as large as 10% of AOD at 354 nm wavelength for Sun photometers with eta = 1.85 degrees. For pyrheliometers (which can have eta up to approximately 2.8 degrees), corrections can be as large as 16% at 354 nm. We find that AOD correction factors are well correlated with AOD wavelength dependence (hence Angstrom exponent). We provide best-fit equations for determining correction factors from Angstrom exponents of uncorrected AOD spectra, and we demonstrate their application to vertical profiles of multiwavelength AOD.

  3. Overview of ACE-Asia Spring 2001 Investigations on Aerosol Radiative Effects and Related Aerosol Properties

    NASA Technical Reports Server (NTRS)

    Russell, Philip B.; Valero, F. P. J.; Flatau, P. J.; Bergin, M.; Holben, B.; Nakajima, T.; Pilewskie, P.; Bergstrom, R.; Hipskind, R. Stephen (Technical Monitor)

    2001-01-01

    depth gradient, with AOD(500 nm) extremes from 0.1 to 1.1. On the Pacific transit from Honolulu to Hachijo AOD(500 nm) averaged 0.2, including increases to 0.4 after several storms, suggesting the strong impact of wind-generated seasalt. The AOD maximum, found in the Sea of Japan, was influenced by dust and anthropogenic sources. (4) In Beijing, single scattering albedo retrieved from AERONET sun-sky radiometry yielded midvisible SSA=0.88 with strong wavelength dependence, suggesting a significant black carbon component. SSA retrieved during dust episodes was approx. 0.90 and variable but wavelength neutral reflecting the presence of urban haze with the dust. Downwind at Anmyon Island SSA was considerably higher, approx. 0.94, but wavelength neutral for dust episodes and spectrally dependent during non dust periods. (5) Satellite retrievals show major aerosol features moving from Asia over the Pacific; however, determining seasonal-average aerosol effects is hampered by sampling frequency and large-scale cloud systems that obscure key parts of aerosol patterns. Preliminary calculations using, satellite-retrieved AOD fields and initial ACE-Asia aerosol properties (including sulfates, soot, and dust) yield clear-sky aerosol radiative effects in the seasonal-average ACE-Asia plume exceeding those of manmade greenhouse gases. Quantifying all-sky direct aerosol radiative effects is complicated by the need to define the height of absorbing aerosols with respect to cloud decks.

  4. Optical, physical and chemical properties of transported African mineral dust aerosols in the Mediterranean region

    NASA Astrophysics Data System (ADS)

    Denjean, Cyrielle; Di Biagio, Claudia; Chevaillier, Servanne; Gaimoz, Cécile; Grand, Noel; Loisil, Rodrigue; Triquet, Sylvain; Zapf, Pascal; Roberts, Greg; Bourrianne, Thierry; Torres, Benjamin; Blarel, Luc; Sellegri, Karine; Freney, Evelyn; Schwarzenbock, Alfons; Ravetta, François; Laurent, Benoit; Mallet, Marc; Formenti, Paola

    2014-05-01

    The transport of mineral dust aerosols is a global phenomenon with strong climate implications. Depending on the travel distance over source regions, the atmospheric conditions and the residence time in the atmosphere, various transformation processes (size-selective sedimentation, mixing, condensation of gaseous species, and weathering) can modify the physical and chemical properties of mineral dust, which, in turn, can change the dust's optical properties. The model predictions of the radiative effect by mineral dust still suffer of the lack of certainty of these properties, and their temporal evolution with transport time. Within the frame of the ChArMex project (Chemistry-Aerosol Mediterranean experiment, http://charmex.lsce.ipsl.fr/), two intensive airborne campaigns (TRAQA, TRansport and Air QuAlity, 18 June - 11 July 2012, and ADRIMED, Aerosol Direct Radiative Impact in the regional climate in the MEDiterranean region, 06 June - 08 July 2013) have been performed over the Central and Western Mediterranean, one of the two major transport pathways of African mineral dust. In this study we have set up a systematic strategy to determine the optical, physical and optical properties of mineral dust to be compared to an equivalent dataset for dust close to source regions in Africa. This study is based on airborne observations onboard the SAFIRE ATR-42 aircraft, equipped with state of the art in situ instrumentation to measure the particle scattering and backscattering coefficients (nephelometer at 450, 550, and 700 nm), the absorption coefficient (PSAP at 467, 530, and 660 nm), the extinction coefficient (CAPS at 530 nm), the aerosol optical depth (PLASMA at 340 to 1640 nm), the size distribution in the extended range 40 nm - 30 µm by the combination of different particle counters (SMPS, USHAS, FSSP, GRIMM) and the chemical composition obtained by filter sampling. The chemistry and transport model CHIMERE-Dust have been used to classify the air masses according to

  5. Sources, Sinks, and Transatlantic Transport of North African Dust Aerosol: A Multimodel Analysis and Comparison With Remote Sensing Data

    NASA Technical Reports Server (NTRS)

    Kim, Dongchul; Chin, Mian; Yu, Hongbin; Diehl, Thomas; Tan, Qian; Kahn, Ralph A.; Tsigaridis, Kostas; Bauer, Susanne E.; Takemura, Toshihiko; Pozzoli, Luca; hide

    2014-01-01

    This study evaluates model-simulated dust aerosols over North Africa and the North Atlantic from five global models that participated in the Aerosol Comparison between Observations and Models phase II model experiments. The model results are compared with satellite aerosol optical depth (AOD) data from Moderate Resolution Imaging Spectroradiometer (MODIS), Multiangle Imaging Spectroradiometer (MISR), and Sea-viewing Wide Field-of-view Sensor, dust optical depth (DOD) derived from MODIS and MISR, AOD and coarse-mode AOD (as a proxy of DOD) from ground-based Aerosol Robotic Network Sun photometer measurements, and dust vertical distributions/centroid height from Cloud Aerosol Lidar with Orthogonal Polarization and Atmospheric Infrared Sounder satellite AOD retrievals. We examine the following quantities of AOD and DOD: (1) the magnitudes over land and over ocean in our study domain, (2) the longitudinal gradient from the dust source region over North Africa to the western North Atlantic, (3) seasonal variations at different locations, and (4) the dust vertical profile shape and the AOD centroid height (altitude above or below which half of the AOD is located). The different satellite data show consistent features in most of these aspects; however, the models display large diversity in all of them, with significant differences among the models and between models and observations. By examining dust emission, removal, and mass extinction efficiency in the five models, we also find remarkable differences among the models that all contribute to the discrepancies of model-simulated dust amount and distribution. This study highlights the challenges in simulating the dust physical and optical processes, even in the best known dust environment, and stresses the need for observable quantities to constrain the model processes.

  6. Dust and biological aerosols from the Sahara and Asia influence precipitation in the western U.S.

    PubMed

    Creamean, Jessie M; Suski, Kaitlyn J; Rosenfeld, Daniel; Cazorla, Alberto; DeMott, Paul J; Sullivan, Ryan C; White, Allen B; Ralph, F Martin; Minnis, Patrick; Comstock, Jennifer M; Tomlinson, Jason M; Prather, Kimberly A

    2013-03-29

    Winter storms in California's Sierra Nevada increase seasonal snowpack and provide critical water resources and hydropower for the state. Thus, the mechanisms influencing precipitation in this region have been the subject of research for decades. Previous studies suggest Asian dust enhances cloud ice and precipitation, whereas few studies consider biological aerosols as an important global source of ice nuclei (IN). Here, we show that dust and biological aerosols transported from as far as the Sahara were present in glaciated high-altitude clouds coincident with elevated IN concentrations and ice-induced precipitation. This study presents the first direct cloud and precipitation measurements showing that Saharan and Asian dust and biological aerosols probably serve as IN and play an important role in orographic precipitation processes over the western United States.

  7. Radiative effects of absorbing aerosols over northeastern India: Observations and model simulations

    NASA Astrophysics Data System (ADS)

    Gogoi, Mukunda M.; Babu, S. Suresh; Moorthy, K. Krishna; Bhuyan, Pradip Kumar; Pathak, Binita; Subba, Tamanna; Chutia, Lakhima; Kundu, Shyam Sundar; Bharali, Chandrakala; Borgohain, Arup; Guha, Anirban; De, Barin Kumar; Singh, Brajamani; Chin, Mian

    2017-01-01

    Multiyear measurements of spectral properties of aerosol absorption are examined over four geographically distinct locations of northeastern India. Results indicated significant spatiotemporal variation in aerosol absorption coefficients (σabs) with highest values in winter and lowest in monsoon. The western parts of the region, close to the outflow of Indo-Gangetic Plains, showed higher values of σabs and black carbon (BC) concentration—mostly associated with fossil fuel combustion. But, the eastern parts showed higher contributions from biomass-burning aerosols, as much as 20-25% to the total aerosol absorption, conspicuously during premonsoon season. This is attributed to a large number of burning activities over the Southeast Asian region, as depicted from Moderate Resolution Imaging Spectroradiometer fire count maps, whose spatial extent and magnitude peaks during March/April. The nearly consistent high values of aerosol index (AI) and layer height from Ozone Monitoring Instrument indicate the presence of absorbing aerosols in the upper atmosphere. The observed seasonality has been captured fairly well by Goddard Chemistry Aerosol Radiation and Transport (GOCART) as well as Weather Research and Forecasting-Chemistry (WRF-Chem) model simulations. The ratio of column-integrated optical depths due to particulate organic matter and BC from GOCART showed good coincidence with satellite-based observations, indicating the increased vertical dispersion of absorbing aerosols, probably by the additional local convection due to higher fire radiative power caused by the intense biomass-burning activities. In the WRF-Chem though underperformed by different magnitude in winter, the values are closer or overestimated near the burnt areas. Atmospheric forcing due to BC was highest ( 30 Wm-2) over the western part associated with the fossil fuel combustion.

  8. An observationally constrained estimate of global dust aerosol optical depth

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Ridley, David A.; Heald, Colette L.; Kok, Jasper F.

    Here, the role of mineral dust in climate and ecosystems has been largely quantified using global climate and chemistry model simulations of dust emission, transport, and deposition. However, differences between these model simulations are substantial, with estimates of global dust aerosol optical depth (AOD) that vary by over a factor of 5. Here we develop an observationally based estimate of the global dust AOD, using multiple satellite platforms, in situ AOD observations and four state-of-the-science global models over 2004–2008. We estimate that the global dust AOD at 550 nm is 0.030 ± 0.005 (1σ), higher than the AeroCom model medianmore » (0.023) and substantially narrowing the uncertainty. The methodology used provides regional, seasonal dust AOD and the associated statistical uncertainty for key dust regions around the globe with which model dust schemes can be evaluated. Exploring the regional and seasonal differences in dust AOD between our observationally based estimate and the four models in this study, we find that emissions in Africa are often overrepresented at the expense of Asian and Middle Eastern emissions and that dust removal appears to be too rapid in most models.« less

  9. An observationally constrained estimate of global dust aerosol optical depth

    DOE PAGES

    Ridley, David A.; Heald, Colette L.; Kok, Jasper F.; ...

    2016-12-06

    Here, the role of mineral dust in climate and ecosystems has been largely quantified using global climate and chemistry model simulations of dust emission, transport, and deposition. However, differences between these model simulations are substantial, with estimates of global dust aerosol optical depth (AOD) that vary by over a factor of 5. Here we develop an observationally based estimate of the global dust AOD, using multiple satellite platforms, in situ AOD observations and four state-of-the-science global models over 2004–2008. We estimate that the global dust AOD at 550 nm is 0.030 ± 0.005 (1σ), higher than the AeroCom model medianmore » (0.023) and substantially narrowing the uncertainty. The methodology used provides regional, seasonal dust AOD and the associated statistical uncertainty for key dust regions around the globe with which model dust schemes can be evaluated. Exploring the regional and seasonal differences in dust AOD between our observationally based estimate and the four models in this study, we find that emissions in Africa are often overrepresented at the expense of Asian and Middle Eastern emissions and that dust removal appears to be too rapid in most models.« less

  10. Retrieving the Height of Smoke and Dust Aerosols by Synergistic Use of VIIRS, OMPS, and CALIOP Observations

    NASA Technical Reports Server (NTRS)

    Lee, Jaehwa; Hsu, N. Christina; Bettenhausen, Corey; Sayer, Andrew M.; Seftor, Colin J.; Jeong, Myeong-Jae

    2015-01-01

    Aerosol Single scattering albedo and Height Estimation (ASHE) algorithm was first introduced in Jeong and Hsu (2008) to provide aerosol layer height as well as single scattering albedo (SSA) for biomass burning smoke aerosols. One of the advantages of this algorithm was that the aerosol layer height can be retrieved over broad areas, which had not been available from lidar observations only. The algorithm utilized aerosol properties from three different satellite sensors, i.e., aerosol optical depth (AOD) and Ångström exponent (AE) from Moderate Resolution Imaging Spectroradiometer (MODIS), UV aerosol index (UVAI) from Ozone Monitoring Instrument (OMI), and aerosol layer height from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). Here, we extend the application of the algorithm to Visible Infrared Imaging Radiometer Suite (VIIRS) and Ozone Mapping and Profiler Suite (OMPS) data. We also now include dust layers as well as smoke. Other updates include improvements in retrieving the AOD of nonspherical dust from VIIRS, better determination of the aerosol layer height from CALIOP, and more realistic input aerosol profiles in the forward model for better accuracy.

  11. Heating Rate of Light Absorbing Aerosols: Time-Resolved Measurements, the Role of Clouds, and Source Identification.

    PubMed

    Ferrero, Luca; Močnik, Griša; Cogliati, Sergio; Gregorič, Asta; Colombo, Roberto; Bolzacchini, Ezio

    2018-03-20

    Light absorbing aerosols (LAA) absorb sunlight and heat the atmosphere. This work presents a novel methodology to experimentally quantify the heating rate (HR) induced by LAA into an atmospheric layer. Multiwavelength aerosol absorption measurements were coupled with spectral measurements of the direct, diffuse and surface reflected radiation to obtain highly time-resolved measurements of HR apportioned in the context of LAA species (black carbon, BC; brown carbon, BrC; dust), sources (fossil fuel, FF; biomass burning, BB), and as a function of cloudiness. One year of continuous and time-resolved measurements (5 min) of HR were performed in the Po Valley. We experimentally determined (1) the seasonal behavior of HR (winter 1.83 ± 0.02 K day -1 ; summer 1.04 ± 0.01 K day -1 ); (2) the daily cycle of HR (asymmetric, with higher values in the morning than in the afternoon); (3) the HR in different sky conditions (from 1.75 ± 0.03 K day -1 in clear sky to 0.43 ± 0.01 K day -1 in complete overcast); (4) the apportionment to different sources: HR FF (0.74 ± 0.01 K day -1 ) and HR BB (0.46 ± 0.01 K day -1 ); and (4) the HR of BrC (HR BrC : 0.15 ± 0.01 K day -1 , 12.5 ± 0.6% of the total) and that of BC (HR BC : 1.05 ± 0.02 K day -1 ; 87.5 ± 0.6% of the total).

  12. Effect of Mineral Dust on Ocean Color Retrievals From Space: A Radiative Transfer Simulation Study

    NASA Astrophysics Data System (ADS)

    Ahmad, Z.; Franz, B. A.

    2016-02-01

    In this paper we examine the effect of mineral aerosols (dust) on the retrieval of ocean colors from space. Mineral aerosols are one of the major components of all aerosols found in the earth's atmosphere. These are mainly soil particles that originate from arid and semiarid regions of the world and are blown away by winds thousands of kilometers away from their source regions. The radii of these aerosols are between 0.1 and 1.0 μm and their resident time in the atmosphere is about 21 days. The primary focus of this paper is to estimate the remote sensing reflectance (Rrs) errors in the presence of absorbing aerosols over ocean. The present study is based on radiative transfer (RT) simulations, and it is particularly relevant to ocean color retrievals from sensors like MODIS, MERIS, VIIRS, and the future PACE/OCI. In the simulations, we have used mineralogy to determine the spectral dependence of aerosol refractive index, and modeled the aerosols to represent dust over Cape Verde (Sal Island). As a part of this study, we will present the results for retrieved aerosol optical thickness (τ), Angstrom exponent (α), and remote sensing reflectance (Rrs) and compare them with similar results for non-absorbing aerosols. In addition, we will show how aerosol layer height affects the ocean color retrievals.

  13. Dust aerosol and optical properties over North Africa simulated with the ALADIN numerical prediction model from 2006 to 2010

    NASA Astrophysics Data System (ADS)

    Mokhtari, M.; Tulet, P.; Fischer, C.; Bouteloup, Y.; Bouyssel, F.; Brachemi, O.

    2015-02-01

    The seasonal cycle and optical properties of mineral dust aerosols in North Africa were simulated for the period from 2006 to 2010 using the numerical atmospheric model ALADIN coupled to the surface scheme SURFEX. The particularity of the simulations is that the major physical processes responsible for dust emission and transport, as well as radiative effects, are taken into account at short timescales and mesoscale resolution. The aim of these simulations is to quantify the dust emission and deposition, locate the major areas of dust emission and establish a climatology of aerosol optical properties in North Africa. The mean monthly Aerosol Optical Thickness (AOT) simulated by ALADIN is compared with the AOTs derived from the standard Dark Target (DT) and Deep Blue (DB) algorithms of the Aqua-MODIS (MODerate resolution Imaging Spectroradiometer) products over North Africa, and with a set of sun photometer measurements located at Banizoumbou, Cinzana, Soroa, Mbour and Capo Verde. The vertical distribution of dust aerosol represented by extinction profiles is also analysed using CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) observations. The annual dust emission simulated by ALADIN over North Africa is 878 Tg year-1. The Bodélé depression appears to be the main area of dust emission in North Africa, with an average estimate of about 21.6 Tg year-1. The simulated AOTs are in good agreement with satellite and sun photometer observations. The positions of the maxima of the modelled AOTs over North Africa match the observed positions, and the ALADIN simulations satisfactorily reproduce the various dust events over the 2006-2010 period. The AOT climatology proposed in this paper provides a solid database of optical properties and consolidates the existing climatology over this region derived from satellites, the AERONET network and Regional Climate Models. Moreover, the three-dimensional distribution of the simulated AOTs also provides information about the

  14. Photochemical aging of light-absorbing secondary organic aerosol material.

    PubMed

    Sareen, Neha; Moussa, Samar G; McNeill, V Faye

    2013-04-11

    Dark reactions of methylglyoxal with NH4(+) in aqueous aerosols yield light-absorbing and surface-active products that can influence the physical properties of the particles. Little is known about how the product mixture and its optical properties will change due to photolysis as well as oxidative aging by O3 and OH in the atmosphere. Here, we report the results of kinetics and product studies of the photochemical aging of aerosols formed by atomizing aqueous solutions of methylglyoxal and ammonium sulfate. Experiments were performed using aerosol flow tube reactors coupled with an aerosol chemical ionization mass spectrometer (Aerosol-CIMS) for monitoring gas- and particle-phase compositions. Particles were also impacted onto quartz windows in order to assess changes in their UV-visible absorption upon oxidation. Photooxidation of the aerosols leads to the formation of small, volatile organic acids including formic acid, acetic acid, and glyoxylic acid. The atmospheric lifetime of these species during the daytime is predicted to be on the order of minutes, with photolysis being an important mechanism of degradation. The lifetime with respect to O3 oxidation was observed to be on the order of hours. O3 oxidation also leads to a net increase in light absorption by the particles due to the formation of additional carbonyl compounds. Our results are consistent with field observations of high brown carbon absorption in the early morning.

  15. Tropospheric Trace Gas Interactions with Aerosols

    NASA Technical Reports Server (NTRS)

    Penner, Joyce E.; Maddrea, George L., Jr. (Technical Monitor)

    2002-01-01

    Tropospheric aerosols are of considerable environmental importance. They modify the radiative budget of Earth by scattering and absorbing radiation, and by providing nuclei for cloud formation. Additionally, they provide surfaces for heterogeneous and multiphase reactions that affect tropospheric chemistry. For example, Dentener and Crutzen (1993) showed that reactions of N2O5 and NO3 with sulfate aerosols may significantly alter the tropospheric concentrations of NO(x), O3, and OH by converting NOx to HNO3 which is rapidly removed by precipitation. Zhang et al. (1994) assumed these same reactions would occur on dust aerosols and showed that dust outbreaks may reduce NO(x) levels by up to 50%. Dentener et al. (1996) studied the possible effect of reactions on dust on sulfate, nitrate, and O3 concentration. Heterogeneous and multiphase reactions on aerosols may also perturb the sulfur cycle the chlorine cycle and the bromine cycle. Because these reactions can release free chlorine and free bromine they might lead to the destruction of ozone in the marine boundary layer that may be important to include in models of tropospheric chemistry. The goal of our proposed work is to examine the role of heterogeneous and multiphase reactions in the tropospheric cycles of reactive nitrogen and sulfur.

  16. Desert dust and anthropogenic aerosol interactions in the Community Climate System Model coupled-carbon-climate model

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Mahowald, Natalie; Rothenberg, D.; Lindsay, Keith

    2011-02-01

    Coupled-carbon-climate simulations are an essential tool for predicting the impact of human activity onto the climate and biogeochemistry. Here we incorporate prognostic desert dust and anthropogenic aerosols into the CCSM3.1 coupled carbon-climate model and explore the resulting interactions with climate and biogeochemical dynamics through a series of transient anthropogenic simulations (20th and 21st centuries) and sensitivity studies. The inclusion of prognostic aerosols into this model has a small net global cooling effect on climate but does not significantly impact the globally averaged carbon cycle; we argue that this is likely to be because the CCSM3.1 model has a small climatemore » feedback onto the carbon cycle. We propose a mechanism for including desert dust and anthropogenic aerosols into a simple carbon-climate feedback analysis to explain the results of our and previous studies. Inclusion of aerosols has statistically significant impacts on regional climate and biogeochemistry, in particular through the effects on the ocean nitrogen cycle and primary productivity of altered iron inputs from desert dust deposition.« less

  17. Inferring Absorbing Organic Carbon Content from AERONET Data

    NASA Technical Reports Server (NTRS)

    Arola, A.; Schuster, G.; Myhre, G.; Kazadzis, S.; Dey, S.; Tripathi, S. N.

    2011-01-01

    Black carbon, light-absorbing organic carbon (often called brown carbon) and mineral dust are the major light-absorbing aerosols. Currently the sources and formation of brown carbon aerosol in particular are not well understood. In this study we estimated globally the amount of light absorbing organic carbon and black carbon from AERONET measurements. We find that the columnar absorbing organic carbon (brown carbon) levels in biomass burning regions of South-America and Africa are relatively high (about 15-20 magnesium per square meters during biomass burning season), while the concentrations are significantly lower in urban areas in US and Europe. However, we estimated significant absorbing organic carbon amounts from the data of megacities of newly industrialized countries, particularly in India and China, showing also clear seasonality with peak values up to 30-35 magnesium per square meters during the coldest season, likely caused by the coal and biofuel burning used for heating. We also compared our retrievals with the modeled organic carbon by global Oslo CTM for several sites. Model values are higher in biomass burning regions than AERONET-based retrievals, while opposite is true in urban areas in India and China.

  18. Radiative Effects of Aerosols Generated from Biomass Burning, Dust Storms, and Forest Fires

    NASA Technical Reports Server (NTRS)

    Christopher Sundar A.; Vulcan, Donna V.; Welch, Ronald M.

    1996-01-01

    Atmospheric aerosol particles, both natural and anthropogenic, are important to the earth's radiative balance. They scatter the incoming solar radiation and modify the shortwave reflective properties of clouds by acting as Cloud Condensation Nuclei (CCN). Although it has been recognized that aerosols exert a net cooling influence on climate (Twomey et al. 1984), this effect has received much less attention than the radiative forcings due to clouds and greenhouse gases. The radiative forcing due to aerosols is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign (Houghton et al. 1990). Atmospheric aerosol particles generated from biomass burning, dust storms and forest fires are important regional climatic variables. A recent study by Penner et al. (1992) proposed that smoke particles from biomass burning may have a significant impact on the global radiation balance. They estimate that about 114 Tg of smoke is produced per year in the tropics through biomass burning. The direct and indirect effects of smoke aerosol due to biomass burning could add up globally to a cooling effect as large as 2 W/sq m. Ackerman and Chung (1992) used model calculations and the Earth Radiation Budget Experiment (ERBE) data to show that in comparison to clear days, the heavy dust loading over the Saudi Arabian peninsula can change the Top of the Atmosphere (TOA) clear sky shortwave and longwave radiant exitance by 40-90 W/sq m and 5-20 W/sq m, respectively. Large particle concentrations produced from these types of events often are found with optical thicknesses greater than one. These aerosol particles are transported across considerable distances from the source (Fraser et al. 1984). and they could perturb the radiative balance significantly. In this study, the regional radiative effects of aerosols produced from biomass burning, dust storms and forest fires are examined using the Advanced Very High Resolution Radiometer (AVHRR) Local Area

  19. Predicting the mineral composition of dust aerosols – Part 1: Representing key processes

    DOE PAGES

    Perlwitz, J. P.; Perez Garcia-Pando, C.; Miller, R. L.

    2015-10-21

    Soil dust aerosols created by wind erosion are typically assigned globally uniform physical and chemical properties within Earth system models, despite known regional variations in the mineral content of the parent soil. Mineral composition of the aerosol particles is important to their interaction with climate, including shortwave absorption and radiative forcing, nucleation of cloud droplets and ice crystals, heterogeneous formation of sulfates and nitrates, and atmospheric processing of iron into bioavailable forms that increase the productivity of marine phytoplankton. Here, aerosol mineral composition is derived by extending a method that provides the composition of a wet-sieved soil. The extension accountsmore » for measurements showing significant differences between the mineral fractions of the wet-sieved soil and the emitted aerosol concentration. For example, some phyllosilicate aerosols are more prevalent at silt sizes, even though they are nearly absent at these diameters in a soil whose aggregates are dispersed by wet sieving. We calculate the emitted mass of each mineral with respect to size by accounting for the disintegration of soil aggregates during wet sieving. These aggregates are emitted during mobilization and fragmentation of the original undispersed soil that is subject to wind erosion. The emitted aggregates are carried far downwind from their parent soil. The soil mineral fractions used to calculate the aggregates also include larger particles that are suspended only in the vicinity of the source. We calculate the emitted size distribution of these particles using a normalized distribution derived from aerosol measurements. In addition, a method is proposed for mixing minerals with small impurities composed of iron oxides. These mixtures are important for transporting iron far from the dust source, because pure iron oxides are more dense and vulnerable to gravitational removal than most minerals comprising dust aerosols. Finally, a

  20. Comparison of characteristics of aerosol during rainy weather and cold air-dust weather in Guangzhou in late March 2012

    NASA Astrophysics Data System (ADS)

    Chen, Huizhong; Wu, Dui; Yu, Jianzhen

    2016-04-01

    Using the data on aerosol observed hourly by Marga ADI 2080 and Grimm 180, we compared the characteristics of aerosol during rainy weather and cold air-dust weather in Guangzhou in late March 2012. The mass concentration of aerosol appeared distinct between the two weather processes. During rainy weather, the mass concentration of PM and total water-soluble components decreased obviously. During cold air-dust weather, the cleaning effect of cold air occurred much more suddenly and about a half day earlier than the dust effect. As a result, the mass concentration of PM and total water-soluble components first dropped dramatically to a below-normal level and then rose gradually to an above-normal level. The ratio of PM2.5/PM10 and PM1/PM10 decreased, suggesting that dust-storm weather mainly brought in coarse particles. The proportion of Ca2+ in the total water-soluble components significantly increased to as high as 50 % because of the effect of dust weather. We further analysed the ionic equilibrium during rainy and cold air-dust weather, and compared it with that during hazy weather during the same period. The aerosol during rainy weather was slightly acidic, whereas that during hazy weather and cold air-dust weather was obviously alkaline, with that during cold air-dust weather being significantly more alkaline. Most of the anions, including SO4 2- and NO3 -, were neutralised by NH4 + during rainy and hazy weather, and by Ca2+ during cold air-dust weather.

  1. Coastal Bacterioplankton Metabolism Is Stimulated Stronger by Anthropogenic Aerosols than Saharan Dust

    PubMed Central

    Marín, Isabel; Nunes, Sdena; Sánchez-Pérez, Elvia D.; Txurruka, Estibalitz; Antequera, Carolina; Sala, Maria M.; Marrasé, Cèlia; Peters, Francesc

    2017-01-01

    In oligotrophic regions, such as the Mediterranean Sea, atmospheric deposition has the potential to stimulate heterotrophic prokaryote growth and production in surface waters, especially during the summer stratification period. Previous studies focused on the role of leaching nutrients from mineral particles of Saharan (S) origin, and were restricted to single locations at given times of the year. In this study, we evaluate the effect of atmospheric particles from diverse sources and with a markedly different chemical composition [S dust and anthropogenic (A) aerosols] on marine planktonic communities from three locations of the northwestern Mediterranean with contrasted anthropogenic footprint. Experiments were also carried out at different times of the year, considering diverse initial conditions. We followed the dynamics of the heterotrophic community and a range of biogeochemical and physiological parameters in six experiments. While the effect of aerosols on bacterial abundance was overall low, bacterial heterotrophic production was up to 3.3 and 2.1 times higher in the samples amended with A and S aerosols, respectively, than in the controls. Extracellular enzymatic activities [leu-aminopeptidase (AMA) and β-glucosidase (β-Gl)] were also enhanced with aerosols, especially from A origin. AMA and β-Gl increased up to 7.1 in the samples amended with A aerosols, and up to 1.7 and 2.1 times, respectively, with S dust. The larger stimulation observed with A aerosols might be attributed to their higher content in nitrate. However, the response was variable depending the initial status of the seawater. In addition, we found that both A and S aerosols stimulated bacterial abundance and metabolism significantly more in the absence of competitors and predators. PMID:29187835

  2. Application of aerosol speciation data as an in situ dust proxy for validation of the Dust Regional Atmospheric Model (DREAM)

    NASA Astrophysics Data System (ADS)

    Shaw, Patrick

    The Dust REgional Atmospheric Model (DREAM) predicts concentrations of mineral dust aerosols in time and space, but validation is challenging with current in situ particulate matter (PM) concentration measurements. Measured levels of ambient PM often contain anthropogenic components as well as windblown mineral dust. In this study, two approaches to model validation were performed with data from preexisting air quality monitoring networks: using hourly concentrations of total PM with aerodynamic diameter less than 2.5 μm (PM 2.5); and using a daily averaged speciation-derived soil component. Validation analyses were performed for point locations within the cities of El Paso (TX), Austin (TX), Phoenix (AZ), Salt Lake City (UT) and Bakersfield (CA) for most of 2006. Hourly modeled PM 2.5 did not validate at all with hourly observations among the sites (combined R < 0.00, N = 24,302 hourly values). Aerosol chemical speciation data distinguished between mineral (soil) dust from anthropogenic ambient PM. As expected, statistically significant improvements in correlation among all stations (combined R = 0.16, N = 343 daily values) were found when the soil component alone was used to validate DREAM. The validation biases that result from anthropogenic aerosols were also reduced using the soil component. This is seen in the reduction of the root mean square error between hourly in situ versus hourly modeled (RMSE hourly = 18.6 μg m -3) and 24-h in situ speciation values versus daily averaged observed (RMSE soil = 12.0 μg m -3). However, the lack of a total reduction in RMSE indicates there is still room for improvement in the model. While the soil component is the theoretical proxy of choice for a dust transport model, the current sparse and infrequent sampling is not ideal for routine hourly air quality forecast validation.

  3. Field observation on secondary organic aerosols during Asian dust storm periods: Formation mechanism of oxalic acid and related compounds on dust surface

    NASA Astrophysics Data System (ADS)

    Wang, Gehui; Cheng, Chunlei; Meng, Jingjing; Huang, Yao; Li, Jianjun; Ren, Yanqin

    2015-07-01

    Chemical evolution of East Asian dust during transpacific transport has been given much attention for inorganic species such as sulfate, nitrate and ammonium. However, the role of organic species during the transport has almost entirely been ignored. To understand the formation mechanism of secondary organic aerosols (SOA) on dust surfaces, this study investigated the concentrations and compositions of dicarboxylic acids, keto-carboxylic acids, α-dicarbonyls and inorganic ions in size-segregated aerosols (9-stages) collected in Xi'an, central China during the two dust storm episodes in the springs of 2009 and 2011 and compared with those in nondust storm periods. During the events the ambient particulate dicarboxylic acids were 932-2240 ng m-3, which are comparable and even higher than those in nondust periods. Molecular compositions of the above SOA are similar to those in nondust periods with oxalic acid being the leading species. In the presence of the dust storms, all the above mentioned SOA species in Xi'an were predominantly enriched on the coarse particles (>2.1 μm), and oxalic acid well correlated with NO3- (R2 = 0.72, p < 0.001) rather than SO42-. This phenomenon differs greatly from the SOA in any other nondust period that is usually characterized by an enrichment of oxalic acid in fine mode and a strong correlation of oxalic acid with SO42-. We propose a formation pathway to explain these observations, in which nitric acid and/or nitrogen oxides react with dust to produce Ca(NO3)2 and form a liquid phase on the surface of dust aerosols via water vapor-absorption of Ca(NO3)2, followed by a partitioning of the gas-phase water-soluble organic precursors (e.g.,glyoxal and methylglyoxal) into the aqueous-phase and a subsequent oxidation into oxalic acid. To the best of our knowledge, we found for the first time the enrichment of glyoxal and methylglyoxal on dust surface. Our data suggest an important role of nitrate in the heterogeneous formation process of

  4. The OMI Aerosol Absorption Product: An A-train application

    NASA Astrophysics Data System (ADS)

    Torres, O.; Jethva, H. T.; Ahn, C.

    2017-12-01

    Because of the uniquely large sensitivity of satellite-measured near-UV radiances to absorption by desert dust, carbonaceous and volcanic ash aerosols, observations by a variety of UV-capable sensors have been routinely used over the last forty years in both qualitative and quantitative applications for estimating the absorption properties of these aerosol types. In this presentation we will discuss a multi-sensor application involving observations from A-train sensors OMI, AIRS and CALIOP for the creation of a 13-year record of aerosol optical depth (AOD) and single scattering albedo (SSA). Determination of aerosol type, in terms of particle size distribution and refractive index, is an important algorithmic step that requires using external information. AIRS CO measurements are used as carbonaceous aerosols tracer to differentiate this aerosol type from desert dust. On the other hand, the height of the absorbing aerosol layer, an important parameter in UV aerosol retrievals, is prescribed using a CALIOP-based climatology. The combined use of these observations in the developments of the OMI long-term AOD/SSA record will be discussed along with an evaluation of retrieval results using independent observations.

  5. The impact of aerosol vertical distribution on aerosol optical depth retrieval using CALIPSO and MODIS data: Case study over dust and smoke regions

    NASA Astrophysics Data System (ADS)

    Wu, Yerong; de Graaf, Martin; Menenti, Massimo

    2017-08-01

    Global quantitative aerosol information has been derived from MODerate Resolution Imaging SpectroRadiometer (MODIS) observations for decades since early 2000 and widely used for air quality and climate change research. However, the operational MODIS Aerosol Optical Depth (AOD) products Collection 6 (C6) can still be biased, because of uncertainty in assumed aerosol optical properties and aerosol vertical distribution. This study investigates the impact of aerosol vertical distribution on the AOD retrieval. We developed a new algorithm by considering dynamic vertical profiles, which is an adaptation of MODIS C6 Dark Target (C6_DT) algorithm over land. The new algorithm makes use of the aerosol vertical profile extracted from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) measurements to generate an accurate top of the atmosphere (TOA) reflectance for the AOD retrieval, where the profile is assumed to be a single layer and represented as a Gaussian function with the mean height as single variable. To test the impact, a comparison was made between MODIS DT and Aerosol Robotic Network (AERONET) AOD, over dust and smoke regions. The results show that the aerosol vertical distribution has a strong impact on the AOD retrieval. The assumed aerosol layers close to the ground can negatively bias the retrievals in C6_DT. Regarding the evaluated smoke and dust layers, the new algorithm can improve the retrieval by reducing the negative biases by 3-5%.

  6. Aerosol contamination survey during dust storm process in Northwestern China using ground, satellite observations and atmospheric modeling data

    NASA Astrophysics Data System (ADS)

    Filonchyk, Mikalai; Yan, Haowen; Shareef, Tawheed Mohammed Elhessin; Yang, Shuwen

    2018-01-01

    The present survey addresses the comprehensive description of geographic locations, transport ways, size, and vertical aerosol distribution during four large dust events which occurred in the Northwest China. Based on the data from 35 ground-based air quality monitoring stations and the satellite data, emission flows for dust events within the period of 2014 to 2017 have been estimated. The data show that maximum peak daily average PM10 and PM2.5 concentrations exceeded 380 and 150 μg/m3, respectively, and the PM2.5/PM10 ratio was ranging within 0.12-0.66. Both satellite data and simulation data of the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) coincide with location and extension of a dust cloud. The Cloud Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) found dust at 0 to 10 km altitude which remained at this level during the most part of its trajectory. The vertical aerosol distribution at a wave of 532 nm total attenuated backscatter coefficient range of 0.0025-0.003 km-1 × sr-1. Moderate Resolution Imaging Spectroradiometer (MODIS) (Terra) Collection 6 Level-3 aerosol products data show that aerosol optical depth (AOD) at pollution epicenters exceeds 1. A comprehensive data survey thus demonstrated that the main sources of high aerosol pollutions in the territory were deserted areas of North and Northwest China as well as the most part of the Republic of Mongolia, where one of the largest deserts, Gobi, extends.

  7. Evaluating aerosol impacts on Numerical Weather Prediction in two extreme dust and biomass-burning events

    NASA Astrophysics Data System (ADS)

    Remy, Samuel; Benedetti, Angela; Jones, Luke; Razinger, Miha; Haiden, Thomas

    2014-05-01

    The WMO-sponsored Working Group on Numerical Experimentation (WGNE) set up a project aimed at understanding the importance of aerosols for numerical weather prediction (NWP). Three cases are being investigated by several NWP centres with aerosol capabilities: a severe dust case that affected Southern Europe in April 2012, a biomass burning case in South America in September 2012, and an extreme pollution event in Beijing (China) which took place in January 2013. At ECMWF these cases are being studied using the MACC-II system with radiatively interactive aerosols. Some preliminary results related to the dust and the fire event will be presented here. A preliminary verification of the impact of the aerosol-radiation direct interaction on surface meteorological parameters such as 2m Temperature and surface winds over the region of interest will be presented. Aerosol optical depth (AOD) verification using AERONET data will also be discussed. For the biomass burning case, the impact of using injection heights estimated by a Plume Rise Model (PRM) for the biomass burning emissions will be presented.

  8. Aerosol Climate Time Series Evaluation In ESA Aerosol_cci

    NASA Astrophysics Data System (ADS)

    Popp, T.; de Leeuw, G.; Pinnock, S.

    2015-12-01

    Within the ESA Climate Change Initiative (CCI) Aerosol_cci (2010 - 2017) conducts intensive work to improve algorithms for the retrieval of aerosol information from European sensors. By the end of 2015 full mission time series of 2 GCOS-required aerosol parameters are completely validated and released: Aerosol Optical Depth (AOD) from dual view ATSR-2 / AATSR radiometers (3 algorithms, 1995 - 2012), and stratospheric extinction profiles from star occultation GOMOS spectrometer (2002 - 2012). Additionally, a 35-year multi-sensor time series of the qualitative Absorbing Aerosol Index (AAI) together with sensitivity information and an AAI model simulator is available. Complementary aerosol properties requested by GCOS are in a "round robin" phase, where various algorithms are inter-compared: fine mode AOD, mineral dust AOD (from the thermal IASI spectrometer), absorption information and aerosol layer height. As a quasi-reference for validation in few selected regions with sparse ground-based observations the multi-pixel GRASP algorithm for the POLDER instrument is used. Validation of first dataset versions (vs. AERONET, MAN) and inter-comparison to other satellite datasets (MODIS, MISR, SeaWIFS) proved the high quality of the available datasets comparable to other satellite retrievals and revealed needs for algorithm improvement (for example for higher AOD values) which were taken into account for a reprocessing. The datasets contain pixel level uncertainty estimates which are also validated. The paper will summarize and discuss the results of major reprocessing and validation conducted in 2015. The focus will be on the ATSR, GOMOS and IASI datasets. Pixel level uncertainties validation will be summarized and discussed including unknown components and their potential usefulness and limitations. Opportunities for time series extension with successor instruments of the Sentinel family will be described and the complementarity of the different satellite aerosol products

  9. Remote Sensing of Aerosol and Aerosol Radiative Forcing of Climate from EOS Terra MODIS Instrument

    NASA Technical Reports Server (NTRS)

    Kaufman, Yoram; Tanre, Didier; Remer, Lorraine; Einaudi, Franco (Technical Monitor)

    2000-01-01

    The recent launch of EOS-Terra into polar orbit has begun to revolutionize remote sensing of aerosol and their effect on climate. Terra has five instruments, two of them,Moderate Resolution Imaging Spectroradiometer (MODIS) and Multiangle Imaging Spectro-Radiometer (MISR) are designed to monitor global aerosol in two different complementary ways. Here we shall discuss the use of the multispectral measurements of MODIS to derive: (1) the global distribution of aerosol load (and optical thickness) over ocean and land; (2) to measure the impact of aerosol on reflection of sunlight to space; and (3) to measure the ability of aerosol to absorb solar radiation. These measurements have direct applications on the understanding of the effect of aerosol on climate, the ability to predict climate change, and on the monitoring of dust episodes and man-made pollution. Principles of remote sensing of aerosol from MODIS will be discussed and first examples of measurements from MODIS will be provided.

  10. Characteristics of aerosol and meteorological parameters during major dust storm events (2005 - 2010) over Beijing, China

    NASA Astrophysics Data System (ADS)

    Zheng, Sheng; Cao, Chunxiang; Singh, Ramesh

    Multi satellite sensors are capable in monitoring dust storm, its path and changes in atmospheric parameters. The present paper discusses aerosol optical properties and meteorological parameters during major dust storm events (2005-2010) over Beijing, China. The back trajectory model shows that the dust is transported from the Inner Mongolia and Mongolia to Beijing. High aerosol optical depth (AOD) and low Ångström exponent (AE) values are observed during dusty days, the average AOD (675 nm) and AE (440-870 nm) during dusty days are 2.33 and 0.06, respectively. The aerosol size distribution (ASD) in coarse mode shows a large increase in the volume during dusty days. The single scattering albedo (SSA) increases with higher wavelength on dusty days, and higher compared to non-dusty days, indicating the presence of high scattering particles due to dust storm events. Characteristics of particles during dusty and non-dusty days are also supported by the real and imaginary parts of refractive index (RI). High air pollution index (API) during dusty days represent poor air quality is a serious health hazard at the time of dust events. The CO volume mixing ratio (COVMR) from Atmospheric Infrared Sounder (AIRS) shows decrease on the ground on dusty days, while the relative humidity (RH) and H _{2}0 mass mixing ratio (H _{2}OMMR) enhance. In addition, due to the dust storm in 2005, enhanced level of water vapor (WV) using Moderate Resolution Imaging Spectroradiometer (MODIS) data is observed in and around Beijing over the dust storms track.

  11. Cavity Ring-Down Measurement of Aerosol Optical Properties During the Asian Dust Above Monterey Experiment and DOE Aerosol Intensive Operating Period

    NASA Technical Reports Server (NTRS)

    Ricci, K.; Strawa, A. W.; Provencal, R.; Castaneda, R.; Bucholtz, A.; Schmid, B.

    2004-01-01

    Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300/Mm with an estimated precision of 0.1/Mm for 1550 nm light and 0.2/Mm for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects. We present comparisons between the Cadenza measurements and those from a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS 14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

  12. Cavity Ring-Down Measurement of Aerosol Optical Properties During the Asian Dust Above Monterey Experiment and DOE Aerosol Intensive Operating Period

    NASA Astrophysics Data System (ADS)

    Ricci, K.; Strawa, A. W.; Provencal, R.; Castaneda, R.; Bucholtz, A.; Schmid, B.

    2003-12-01

    Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300 Mm-1 with an estimated precision of 0.1 Mm-1 for 1550 nm light and 0.2 Mm-1 for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects. We present comparisons between the Cadenza measurements and those from a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

  13. Global dust sources detection using MODIS Deep Blue Collection 6 aerosol products

    NASA Astrophysics Data System (ADS)

    Pérez García-Pando, C.; Ginoux, P. A.

    2015-12-01

    Our understanding of the global dust cycle is limited by a dearth of information about dust sources, especially small-scale features which could account for a large fraction of global emissions. Remote sensing sensors are the most useful tool to locate dust sources. These sensors include microwaves, visible channels, and lidar. On the global scale, major dust source regions have been identified using polar orbiting satellite instruments. The MODIS Deep Blue algorithm has been particularly useful to detect small-scale sources such as floodplains, alluvial fans, rivers, and wadis , as well as to identify anthropogenic sources from agriculture. The recent release of Collection 6 MODIS aerosol products allows to extend dust source detection to the entire land surfaces, which is quite useful to identify mid to high latitude dust sources and detect not only dust from agriculture but fugitive dust from transport and industrial activities. This presentation will overview the advantages and drawbacks of using MODIS Deep Blue for dust detection, compare to other instruments (polar orbiting and geostationary). The results of Collection 6 with a new dust screening will be compared against AERONET. Applications to long range transport of anthropogenic dust will be presented.

  14. Investigation of the seasonal variations of aerosol physicochemical properties and their impact on cloud condensation nuclei number concentration

    NASA Astrophysics Data System (ADS)

    Logan, Timothy S.

    Aerosols are among the most complex yet widely studied components of the atmosphere not only due to the seasonal variability of their physical and chemical properties but also their effects on climate change. The three main aerosol types that are known to affect the physics and chemistry of the atmosphere are: mineral dust, anthropogenic pollution, and biomass burning aerosols. In order to understand how these aerosols affect the atmosphere, this dissertation addresses the following three scientific questions through a combination of surface and satellite observations: SQ1: What are the seasonal and regional variations of aerosol physico-chemical properties at four selected Asian sites? SQ2: How do these aerosol properties change during transpacific and intra-continental long range transport? SQ3: What are the impacts of aerosol properties on marine boundary layer cloud condensation nuclei number concentration? This dissertation uses an innovative approach to classify aerosol properties by region and season to address SQ1. This is useful because this method provides an additional dimension when investigating the physico-chemical properties of aerosols by linking a regional and seasonal dependence to both the aerosol direct and indirect effects. This method involves isolating the aerosol physico-chemical properties into four separate regions using AERONET retrieved Angstrom exponent (AEAOD) and single scattering co-albedo (o oabs) to denote aerosol size and absorptive properties. The aerosols events are then clustered by season. The method is first applied to four AERONET sites representing single mode aerosol dominant regions: weakly absorbing pollution (NASA Goddard), strongly absorbing pollution (Mexico City), mineral dust (Solar Village), and biomass burning smoke (Alta Floresta). The method is then applied to four Asian sites that represent complicated aerosol components. There are strong regional and seasonal influences of the four aerosol types over the

  15. Absorption Properties of Mediterranean Aerosols Obtained from Multi-year Ground-based and Satellite Remote Sensing Observations

    NASA Technical Reports Server (NTRS)

    Mallet, M.; Dubovik, O.; Nabat, P.; Dulac, F.; Kahn, R.; Sciare, J.; Paronis, D.; Leon, J. F.

    2013-01-01

    Aerosol absorption properties are of high importance to assess aerosol impact on regional climate. This study presents an analysis of aerosol absorption products obtained over the Mediterranean Basin or land stations in the region from multi-year ground-based AERONET and satellite observations with a focus on the Absorbing Aerosol Optical Depth (AAOD), Single Scattering Albedo (SSA) and their spectral dependence. The AAOD and Absorption Angstrom Exponent (AAE) data set is composed of daily averaged AERONET level 2 data from a total of 22 Mediterranean stations having long time series, mainly under the influence of urban-industrial aerosols and/or soil dust. This data set covers the 17 yr period 1996-2012 with most data being from 2003-2011 (approximately 89 percent of level-2 AAOD data). Since AERONET level-2 absorption products require a high aerosol load (AOD at 440 nm greater than 0.4), which is most often related to the presence of desert dust, we also consider level-1.5 SSA data, despite their higher uncertainty, and filter out data with an Angstrom exponent less than 1.0 in order to study absorption by carbonaceous aerosols. The SSA data set includes both AERONET level-2 and satellite level-3 products. Satellite-derived SSA data considered are monthly level 3 products mapped at the regional scale for the spring and summer seasons that exhibit the largest aerosol loads. The satellite SSA dataset includes the following products: (i) Multi-angle Imaging SpectroRadiometer (MISR) over 2000-2011, (ii) Ozone Monitoring Instrument (OMI) near-UV algorithm over 2004-2010, and (iii) MODerate resolution Imaging Spectroradiometer (MODIS) Deep-Blue algorithm over 2005-2011, derived only over land in dusty conditions. Sun-photometer observations show that values of AAOD at 440 nm vary between 0.024 +/- 0.01 (resp. 0.040 +/- 0.01) and 0.050 +/- 0.01 (0.055 +/- 0.01) for urban (dusty) sites. Analysis shows that the Mediterranean urban-industrial aerosols appear "moderately

  16. Modelling soil dust aerosol in the Bodélé depression during the BoDEx campaign

    NASA Astrophysics Data System (ADS)

    Tegen, I.; Heinold, B.; Todd, M.; Helmert, J.; Washington, R.; Dubovik, O.

    2006-05-01

    We present regional model simulations of the dust emission events during the Bodélé Dust Experiment (BoDEx) that was carried out in February and March 2005 in Chad. A box model version of the dust emission model is used to test different input parameters for the emission model, and to compare the dust emissions computed with observed wind speeds to those calculated with wind speeds from the regional model simulation. While field observations indicate that dust production occurs via self-abrasion of saltating diatomite flakes in the Bodélé, the emission model based on the assumption of dust production by saltation and using observed surface wind speeds as input parameters reproduces observed dust optical thicknesses well. Although the peak wind speeds in the regional model underestimate the highest wind speeds occurring on 10-12 March 2005, the spatio-temporal evolution of the dust cloud can be reasonably well reproduced by this model. Dust aerosol interacts with solar and thermal radiation in the regional model; it is responsible for a decrease in maximum daytime temperatures by about 5 K at the beginning the dust storm on 10 March 2005. This direct radiative effect of dust aerosol accounts for about half of the measured temperature decrease compared to conditions on 8 March. Results from a global dust model suggest that the dust from the Bodélé is an important contributor to dust crossing the African Savannah region towards the Gulf of Guinea and the equatorial Atlantic, where it can contribute up to 40% to the dust optical thickness.

  17. Modelling soil dust aerosol in the Bodélé depression during the BoDEx campaign

    NASA Astrophysics Data System (ADS)

    Tegen, I.; Heinold, B.; Todd, M.; Helmert, J.; Washington, R.; Dubovik, O.

    2006-09-01

    We present regional model simulations of the dust emission events during the Bodélé Dust Experiment (BoDEx) that was carried out in February and March 2005 in Chad. A box model version of the dust emission model is used to test different input parameters for the emission model, and to compare the dust emissions computed with observed wind speeds to those calculated with wind speeds from the regional model simulation. While field observations indicate that dust production occurs via self-abrasion of saltating diatomite flakes in the Bodélé, the emission model based on the assumption of dust production by saltation and using observed surface wind speeds as input parameters reproduces observed dust optical thicknesses well. Although the peak wind speeds in the regional model underestimate the highest wind speeds occurring on 10-12 March 2005, the spatio-temporal evolution of the dust cloud can be reasonably well reproduced by this model. Dust aerosol interacts with solar and thermal radiation in the regional model; it is responsible for a decrease in maximum daytime temperatures by about 5 K at the beginning the dust storm on 10 March 2005. This direct radiative effect of dust aerosol accounts for about half of the measured temperature decrease compared to conditions on 8 March. Results from a global dust model suggest that the dust from the Bodélé is an important contributor to dust crossing the African Savannah region towards the Gulf of Guinea and the equatorial Atlantic, where it can contribute up to 40% to the dust optical thickness.

  18. Light-absorbing oligomer formation in secondary organic aerosol from reactive uptake of isoprene epoxydiols.

    PubMed

    Lin, Ying-Hsuan; Budisulistiorini, Sri Hapsari; Chu, Kevin; Siejack, Richard A; Zhang, Haofei; Riva, Matthieu; Zhang, Zhenfa; Gold, Avram; Kautzman, Kathryn E; Surratt, Jason D

    2014-10-21

    Secondary organic aerosol (SOA) produced from reactive uptake and multiphase chemistry of isoprene epoxydiols (IEPOX) has been found to contribute substantially (upward of 33%) to the fine organic aerosol mass over the Southeastern U.S. Brown carbon (BrC) in rural areas of this region has been linked to secondary sources in the summer when the influence of biomass burning is low. We demonstrate the formation of light-absorbing (290 < λ < 700 nm) SOA constituents from reactive uptake of trans-β-IEPOX onto preexisting sulfate aerosols as a potential source of secondary BrC. IEPOX-derived BrC generated in controlled chamber experiments under dry, acidic conditions has an average mass absorption coefficient of ∼ 300 cm(2) g(-1). Chemical analyses of SOA constituents using UV-visible spectroscopy and high-resolution mass spectrometry indicate the presence of highly unsaturated oligomeric species with molecular weights separated by mass units of 100 (C5H8O2) and 82 (C5H6O) coincident with the observations of enhanced light absorption, suggesting such oligomers as chromophores, and potentially explaining one source of humic-like substances (HULIS) ubiquitously present in atmospheric aerosol. Similar light-absorbing oligomers were identified in fine aerosol collected in the rural Southeastern U.S., supporting their atmospheric relevance and revealing a previously unrecognized source of oligomers derived from isoprene that contributes to ambient fine aerosol mass.

  19. Mixing states of aerosols over four environmentally distinct atmospheric regimes in Asia: coastal, urban, and industrial locations influenced by dust.

    PubMed

    Ramachandran, S; Srivastava, Rohit

    2016-06-01

    Mixing can influence the optical, physical, and chemical characteristics of aerosols, which in turn can modify their life cycle and radiative effects. Assumptions on the mixing state can lead to uncertain estimates of aerosol radiative effects. To examine the effect of mixing on the aerosol characteristics, and their influence on radiative effects, aerosol mixing states are determined over four environmentally distinct locations (Karachi, Gwangju, Osaka, and Singapore) in Asia, an aerosol hot spot region, using measured spectral aerosol optical properties and optical properties model. Aerosol optical depth (AOD), single scattering albedo (SSA), and asymmetry parameter (g) exhibit spectral, spatial, and temporal variations. Aerosol mixing states exhibit large spatial and temporal variations consistent with aerosol characteristics and aerosol type over each location. External mixing of aerosol species is unable to reproduce measured SSA over Asia, thus providing a strong evidence that aerosols exist in mixed state. Mineral dust (MD) (core)-Black carbon (BC) (shell) is one of the most preferred aerosol mixing states. Over locations influenced by biomass burning aerosols, BC (core)-water soluble (WS, shell) is a preferred mixing state, while dust gets coated by anthropogenic aerosols (BC, WS) over urban regions influenced by dust. MD (core)-sea salt (shell) mixing is found over Gwangju corroborating the observations. Aerosol radiative forcing exhibits large seasonal and spatial variations consistent with features seen in aerosol optical properties and mixing states. TOA forcing is less negative/positive for external mixing scenario because of lower SSA. Aerosol radiative forcing in Karachi is a factor of 2 higher when compared to Gwangju, Osaka, and Singapore. The influence of g on aerosol radiative forcing is insignificant. Results emphasize that rather than prescribing one single aerosol mixing state in global climate models regionally and temporally varying aerosol

  20. Remote sensing of soot carbon - Part 1: Distinguishing different absorbing aerosol species

    NASA Astrophysics Data System (ADS)

    Schuster, G. L.; Dubovik, O.; Arola, A.

    2016-02-01

    We describe a method of using the Aerosol Robotic Network (AERONET) size distributions and complex refractive indices to retrieve the relative proportion of carbonaceous aerosols and free iron minerals (hematite and goethite). We assume that soot carbon has a spectrally flat refractive index and enhanced imaginary indices at the 440 nm wavelength are caused by brown carbon or hematite. Carbonaceous aerosols can be separated from dust in imaginary refractive index space because 95 % of biomass burning aerosols have imaginary indices greater than 0.0042 at the 675-1020 nm wavelengths, and 95 % of dust has imaginary refractive indices of less than 0.0042 at those wavelengths. However, mixtures of these two types of particles can not be unambiguously partitioned on the basis of optical properties alone, so we also separate these particles by size. Regional and seasonal results are consistent with expectations. Monthly climatologies of fine mode soot carbon are less than 1.0 % by volume for West Africa and the Middle East, but the southern African and South American biomass burning sites have peak values of 3.0 and 1.7 %. Monthly averaged fine mode brown carbon volume fractions have a peak value of 5.8 % for West Africa, 2.1 % for the Middle East, 3.7 % for southern Africa, and 5.7 % for South America. Monthly climatologies of free iron volume fractions show little seasonal variability, and range from about 1.1 to 1.7 % for coarse mode aerosols in all four study regions. Finally, our sensitivity study indicates that the soot carbon retrieval is not sensitive to the component refractive indices or densities assumed for carbonaceous and free iron aerosols, and the retrieval differs by only 15.4 % when these parameters are altered from our chosen baseline values. The total uncertainty of retrieving soot carbon mass is ˜ 50 % (when uncertainty in the AERONET product and mixing state is included in the analysis).

  1. Impact of aerosols, dust, water vapor and clouds on fair weather PG and implications for the Carnegie curve

    NASA Astrophysics Data System (ADS)

    Kourtidis, Konstantinos; Georgoulias, Aristeidis

    2017-04-01

    We studied the impact of anthropogenic aerosols, fine mode natural aerosols, Saharan dust, atmospheric water vapor, cloud fraction, cloud optical depth and cloud top height on the magnitude of fair weather PG at the rural station of Xanthi. Fair weather PG was measured in situ while the other parameters were obtained from the MODIS instrument onboard the Terra and Aqua satellites. All of the above parameteres were found to impact fair weather PG magnitude. Regarding aerosols, the impact was larger for Saharan dust and fine mode natural aerosols whereas regarding clouds the impact was larger for cloud fraction while less than that of aerosols. Water vapour and ice precipitable water were also found to influence fair weather PG. Since aerosols and water are ubiquitous in the atmosphere and exhibit large spatial and temporal variability, we postulate that our understanding of the Carnegie curve might need revision.

  2. Evidence of a Weakly Absorbing Intermediate Mode of Aerosols in AERONET Data from Saharan and Sahelian Sites

    NASA Technical Reports Server (NTRS)

    Gianelli, Scott M.; Lacis, Andrew A.; Carlson, Barbara E.; Hameed, Sultan

    2013-01-01

    Accurate retrievals of aerosol size distribution are necessary to estimate aerosols' impact on climate and human health. The inversions of the Aerosol Robotic Network (AERONET) usually retrieve bimodal distributions. However, when the inversion is applied to Saharan and Sahelian dust, an additional mode of intermediate size between the coarse and fine modes is sometimes seen. This mode explains peculiarities in the behavior of the Angstrom exponent, along with the fine mode fraction retrieved using the spectral deconvolution algorithm, observed in a March 2006 dust storm. For this study, 15 AERONET sites in northern Africa and on the Atlantic are examined to determine the frequency and properties of the intermediate mode. The mode is observed most frequently at Ilorin in Nigeria. It is also observed at Capo Verde and multiple sites located within the Sahel but much less frequently at sites in the northern Sahara and the Canary Islands. The presence of the intermediate mode coincides with increases in Angstrom exponent, fine mode fraction, single-scattering albedo, and to a lesser extent percent sphericity. The Angstrom exponent decreases with increasing optical depth at most sites when the intermediate mode is present, but the fine mode fraction does not. Single-scattering albedo does not steadily decrease with fine mode fraction when the intermediate mode is present, as it does in typical mixtures of dust and biomass-burning aerosols. Continued investigation is needed to further define the intermediate mode's properties, determine why it differs from most Saharan dust, and identify its climate and health effects.

  3. Relationships between Personal Measurements of 'Total' Dust, Respirable, Thoracic, and Inhalable Aerosol Fractions in the Cement Production Industry.

    PubMed

    Notø, Hilde P; Nordby, Karl-Christian; Eduard, Wijnand

    2016-05-01

    The aims of this study were to examine the relationships and establish conversion factors between 'total' dust, respirable, thoracic, and inhalable aerosol fractions measured by parallel personal sampling on workers from the production departments of cement plants. 'Total' dust in this study refers to aerosol sampled by the closed face 37-mm Millipore filter cassette. Side-by-side personal measurements of 'total' dust and respirable, thoracic, and inhalable aerosol fractions were performed on workers in 17 European and Turkish cement plants. Simple linear and mixed model regressions were used to model the associations between the samplers. The total number of personal samples collected on 141 workers was 512. Of these 8.4% were excluded leaving 469 for statistical analysis. The different aerosol fractions contained from 90 to 130 measurements and-side-by side measurements of all four aerosol fractions were collected on 72 workers.The median ratios between observed results of the respirable, 'total' dust, and inhalable fractions relative to the thoracic aerosol fractions were 0.51, 2.4, and 5.9 respectively. The ratios between the samplers were not constant over the measured concentration range and were best described by regression models. Job type, position of samplers on left or right shoulder and plant had no substantial effect on the ratios. The ratios between aerosol fractions changed with different air concentrations. Conversion models for estimation of the fractions were established. These models explained a high proportion of the variance (74-91%) indicating that they are useful for the estimation of concentrations based on measurements of a different aerosol fraction. The calculated uncertainties at most observed concentrations were below 30% which is acceptable for comparison with limit values (EN 482, 2012). The cement industry will therefore be able to predict the health related aerosol fractions from their former or future measurements of one of the

  4. Modeled Response of Greenland Climate to the Presence of Biomass Burning-Based Absorbing Aerosols in the Atmosphere and Snow

    NASA Astrophysics Data System (ADS)

    Ward, J. L.; Flanner, M.; Bergin, M. H.; Courville, Z.; Dibb, J. E.; Polashenski, C.; Soja, A. J.; Strellis, B. M.; Thomas, J. L.

    2016-12-01

    Combustion of biomass material results in the emission of microscopic particles, some of which absorb incoming solar radiation. Including black carbon (BC), these absorbing species can affect regional climate through changes in the local column energy budgets, cloud direct and indirect effects, and atmospheric dynamical processes. The cryosphere, which consists of both snow and ice, is unusually susceptible to changes in radiation due to its characteristically high albedo. As the largest element of the cryosphere in the Northern Hemisphere, the Greenland Ice Sheet (GrIS) covers most of Greenland's terrestrial surface and, if subjected to the increased presence of light-absorbing impurities, could experience enhanced melt. A particularly enhanced melt episode of the GrIS occurred during July 2012; at the same time, large-scale biomass burning events were observed in Eurasia and North America. Observations showed that, at the same time, single-scattering albedo (SSA) was lower than average while aerosol optical depth (AOD) was high for the Greenland region. In this study, we apply idealized climate simulations to analyze how various aspects of Greenland's climate are affected by the enhanced presence of particulate matter in the atmospheric and on the surface of the GrIS. We employ the Community Earth System Model (CESM) with prescribed sea surface temperatures and active land and atmospheric components. Using four sets of modeling experiments, we perturb 1) only AOD, 2) only SSA, 3) mass mixing ratios of BC and dust in snow, and 4) both AOD and in-snow impurity concentrations. The chosen values for each of these modeling experiments are based on field measurements taken in 2011 (AOD, SSA) and the summers of 2012-2014 (mass mixing ratios of BC and dust). Comparing the results of these experiments provides information on how the overall climate of Greenland could be affected by large biomass burning events.

  5. Multi-wavelength aerosol light absorption measurements in the Amazon rainforest

    NASA Astrophysics Data System (ADS)

    Saturno, Jorge; Chi, Xuguang; Pöhlker, Christopher; Morán, Daniel; Ditas, Florian; Massabò, Dario; Prati, Paolo; Rizzo, Luciana; Artaxo, Paulo; Andreae, Meinrat

    2015-04-01

    The most important light-absorbing aerosol is black carbon (BC), which is emitted by incomplete combustion of fossil fuels and biomass. BC is considered the second anthropogenic contributor to global warming. Beyond BC, other aerosols like some organics, dust, and primary biological aerosol particles are able to absorb radiation. In contrast to BC, the light absorption coefficient of these aerosols is wavelength dependent. Therefore, multi-wavelength measurements become important in environments where BC is not the predominant light-absorbing aerosol like in the Amazon. The Amazon Tall Tower Observatory (ATTO) site is located in the remote Amazon rainforest, one of the most pristine continental sites in the world during the wet season. In the dry season, winds coming from the southern hemisphere are loaded with biomass burning aerosol particles originated by farming-related deforestation. BC and aerosol number concentration data from the last two years indicate this is the most polluted period. Two different techniques have been implemented to measure the light absorption at different wavelengths; one of them is the 7-wavelengths Aethalometer, model AE30, an instrument that measures the light attenuation on a filter substrate and requires multiple scattering and filter-loading corrections to retrieve the light absorption coefficient. The other method is an offline technique, the Multi-Wavelength Absorbance Analysis (MWAA), which is able to measure reflectance and absorbance by aerosols collected on a filter and, by means of a radiative model, can retrieve the light absorption coefficient. Filters collected during May-September 2014, comprehending wet-to-dry transition and most of the dry season, were analyzed. The results indicate that the Absorption Ångström Exponent (AAE), a parameter that is directly proportional to the wavelength dependence of the aerosol light absorption, is close to 1.0 during the transition period and slightly decreases in the beginning of

  6. The variation of characteristics and formation mechanisms of aerosols in dust, haze, and clear days in Beijing

    NASA Astrophysics Data System (ADS)

    Wang, Ying; Zhuang, Guoshun; Sun, Yele; An, Zhisheng

    A 4-year campaign from 2001 to 2004 monitoring PM 2.5 and TSP in the spring season in urban Beijing, China was performed to study the variation of characteristics and the different formation mechanisms of aerosols in dust, haze, and clear days. A total of 315 aerosol samples were collected and used in this study. The aerosols were more basic in dust days and more acidic in haze days. The ions presented in the order of SO42->Ca 2+≫ NO3->Cl -> NH4+>Na + in dust days, and of SO42-> NO3-> NH4+≫Cl ->Ca 2+>K + in haze days. Ions has been classified into three groups, "Na +, Mg 2+, Ca 2+", "K +, SO42-, Cl -", and " NO3-, NH4+", representing crust, pollution-crust, and pollution species, respectively. Crust and pollution ions were the main ion fractions in dust and haze days, respectively. The variation of Ca 2+/Al showed that the increase of dust in dust and haze days was from soil and construction, respectively. "CaCO 3, CaSO 4, and (NH 4) 2SO 4" and "(NH 4) 2SO 4, NH 4NO 3, and Ca(NO 3) 2" were the major species in dust and haze days, respectively. The formation of CaSO 4 on airborne soil particles and the formation of (NH 4) 2SO 4 and NH 4NO 3 were the predominant pathways of sulfate and nitrate formations in dust and haze days, respectively. Sulfate might be mainly formed through heterogeneous reactions in the aqueous surface layer on the pre-existing particles, while nitrate mainly through homogeneous gas-phase reactions in the spring season in Beijing. The formation of sulfate and nitrate was accelerated in dust and haze days.

  7. Spectral Absorption of Solar Radiation by Aerosols during ACE-Asia

    NASA Technical Reports Server (NTRS)

    Bergstrom, R. W.; Pilewskie, P.; Pommier, J.; Rabbette, M.; Russell, P. B.; Schmid, B.; Redermann, J.; Higurashi, A.; Nakajima, T.; Quinn, P. K.

    2004-01-01

    As part of the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia), the upward and downward spectral solar radiant fluxes were measured with the Spectral Solar Flux Radiometer (SSFR), and the aerosol optical depth was measured with the Ames Airborne Tracking Sunphotometer (AATS-14) aboard the Center for INterdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS) Twin Otter aircraft. IN this paper, we examine the data obtained for two cases: a moderately thick aerosol layer, 12 April, and a relatively thin aerosol case, 16 April 2001. ON both days, the Twin Otter flew vertical profiles in the Korean Strait southeast of Gosan Island. For both days we determine the aerosol spectral absorption of the layer and estimate the spectral aerosol absorption optical depth and single-scattering albedo. The results for 12 April show that the single-scattering albedo increases with wavelength from 0.8 at 400 nm to 0.95 at 900 nm and remains essentially constant from 950 to 1700 nm. On 16 April the amount of aerosol absorption was very low; however, the aerosol single-scattering albedo appears to decrease slightly with wavelength in the visible region. We interpret these results in light of the two absorbing aerosol species observed during the ACE-asia study: mineral dust and black carbon. The results for 12 April are indicative of a mineral dust-black carbon mixture. The 16 April results are possibly caused by black carbon mixed with nonabsorbing pollution aerosols. For the 12 April case we attempt to estimate the relative contributions of the black carbon particles and the mineral dust particles. We compare our results with other estimates of the aerosol properties from a Sea-Viewing Wide Field-of-View Sensor (SeaWiFS) satellite analysis and aerosol measurements made aboard the Twin Otter, aboard the National Oceanic and Atmospheric Administration Ronald H Brown ship, and at ground sites in Gosan and Japan. The results indicate a relatively complicated aerosol

  8. Saharan dust as a causal factor of hemispheric asymmetry in aerosols and cloud cover over the tropical Atlantic Ocean

    DOE PAGES

    Kishcha, Pavel; Da Sliva, Arlindo; Starobinets, Boris; ...

    2015-07-09

    Meridional distribution of aerosol optical thickness (AOT) over the tropical Atlantic Ocean (30°N – 30°S) was analyzed to assess seasonal variations of meridional AOT asymmetry. Ten-year MERRA Aerosol Reanalysis (MERRAero) data (July 2002 – June 2012) confirms that the Sahara desert emits a significant amount of dust into the atmosphere over the Atlantic Ocean. Only over the Atlantic Ocean did MERRAero show that desert dust dominates other aerosol species and is responsible for meridional aerosol asymmetry between the tropical North and South Atlantic. Over the 10-year period under consideration, both MISR measurements and MERRAero data showed a pronounced meridional AOTmore » asymmetry. The meridional AOT asymmetry, characterized by the hemispheric ratio (RAOT) of AOT averaged separately over the North and over the South Atlantic, was about 1.7. Seasonally, meridional AOT asymmetry over the Atlantic was the most pronounced between March and July, when dust presence is maximal (RAOT ranged from 2 to 2.4). There was no noticeable meridional aerosol asymmetry in total AOT from September to October. During this period the contribution of carbonaceous aerosols to total AOT in the South Atlantic was comparable to the contribution of dust aerosols to total AOT in the North Atlantic. During the same 10-year period, MODIS cloud fraction (CF) data showed that there was no noticeable asymmetry in meridional CF distribution in different seasons (the hemispheric ratio of CF ranged from 1.0 to 1.2). MODIS CF data illustrated significant cloud cover (CF of 0.7 – 0.9) with limited precipitation ability along the Saharan Air Layer.« less

  9. Aerosol Climate Time Series in ESA Aerosol_cci

    NASA Astrophysics Data System (ADS)

    Popp, Thomas; de Leeuw, Gerrit; Pinnock, Simon

    2016-04-01

    Within the ESA Climate Change Initiative (CCI) Aerosol_cci (2010 - 2017) conducts intensive work to improve algorithms for the retrieval of aerosol information from European sensors. Meanwhile, full mission time series of 2 GCOS-required aerosol parameters are completely validated and released: Aerosol Optical Depth (AOD) from dual view ATSR-2 / AATSR radiometers (3 algorithms, 1995 - 2012), and stratospheric extinction profiles from star occultation GOMOS spectrometer (2002 - 2012). Additionally, a 35-year multi-sensor time series of the qualitative Absorbing Aerosol Index (AAI) together with sensitivity information and an AAI model simulator is available. Complementary aerosol properties requested by GCOS are in a "round robin" phase, where various algorithms are inter-compared: fine mode AOD, mineral dust AOD (from the thermal IASI spectrometer, but also from ATSR instruments and the POLDER sensor), absorption information and aerosol layer height. As a quasi-reference for validation in few selected regions with sparse ground-based observations the multi-pixel GRASP algorithm for the POLDER instrument is used. Validation of first dataset versions (vs. AERONET, MAN) and inter-comparison to other satellite datasets (MODIS, MISR, SeaWIFS) proved the high quality of the available datasets comparable to other satellite retrievals and revealed needs for algorithm improvement (for example for higher AOD values) which were taken into account for a reprocessing. The datasets contain pixel level uncertainty estimates which were also validated and improved in the reprocessing. For the three ATSR algorithms the use of an ensemble method was tested. The paper will summarize and discuss the status of dataset reprocessing and validation. The focus will be on the ATSR, GOMOS and IASI datasets. Pixel level uncertainties validation will be summarized and discussed including unknown components and their potential usefulness and limitations. Opportunities for time series extension

  10. Modeling and observations of dust aerosols during the North American Monsoon

    NASA Astrophysics Data System (ADS)

    Arellano, A. F.; Raman, A.; Brost, J.; Sorooshian, A.

    2016-12-01

    Intense dust storms during North American Monsoon (NAM) pose a significant threat to local/regional air quality, economy, and public health. Convection-driven storms (or haboobs) in Arizona and in the southwest US have been given far less attention compared to those in Africa and Middle East. Blowing dusts from these haboobs typically lasts for 3-6 hours and accumulate more than 1000 µg m-3 of PM10 in the atmosphere. However, it is not clear whether haboobs are increasing in intensity and/or frequency in Arizona. Here, we address two science questions: 1) Do haboobs impact the observed trends in aerosol abundance in the NAM region?, 2) What are our current capabilities and limitations in understanding, monitoring, and assessing haboobs and their impacts? For 1), we calculated the trends of enhancements in aerosol optical depth (AOD) from Terra MODIS over dust hotspots in the NAM alley and and surrounding region (dust cluster). Both show similar decreasing trends before the monsoon. However, during the monsoon, a decreasing trend in AOD is more prominent in the dust cluster than in NAM alley. We attribute this to an apparent modulation of dust in the NAM alley by haboobs. Despite increase in rainfall during this period, we infer that the increase in dust sources in the NAM alley obscures the decreasing AOD trend. For 2), we conducted simulations simulations of these haboobs using WRF-Chem with GOCART AFWA scheme at convective resolving scales ( 1 km). Our case study for the 5 July 2011 haboob indicate that the downbursts occurred near Tucson and generated diverging high intensity winds, resulting to cold pools propagating towards Phoenix. We find that WRF-Chem captures the timing of the haboob but severely underestimates the magnitude of dust concentrations that reached as high as 2000 µg m-3 at USEPA Phoenix stations. The impact of the haboob was seen as far as 350 km northwest of Phoenix at an altitude of 2-4 km on 6 July. We find two major limitations in our

  11. Three-dimensional dust aerosol distribution and extinction climatology over northern Africa simulated with the ALADIN numerical prediction model from 2006 to 2010

    NASA Astrophysics Data System (ADS)

    Mokhtari, M.; Tulet, P.; Fischer, C.; Bouteloup, Y.; Bouyssel, F.; Brachemi, O.

    2015-08-01

    The seasonal cycle and optical properties of mineral dust aerosols in northern Africa were simulated for the period from 2006 to 2010 using the numerical atmospheric model ALADIN (Aire Limitée Adaptation dynamique Développement InterNational) coupled to the surface scheme SURFEX (SURFace EXternalisée). The particularity of the simulations is that the major physical processes responsible for dust emission and transport, as well as radiative effects, are taken into account on short timescales and at mesoscale resolution. The aim of these simulations is to quantify the dust emission and deposition, locate the major areas of dust emission and establish a climatology of aerosol optical properties in northern Africa. The mean monthly aerosol optical thickness (AOT) simulated by ALADIN is compared with the AOTs derived from the standard Dark Target (DT) and Deep Blue (DB) algorithms of the Aqua-MODIS (MODerate resolution Imaging Spectroradiometer) products over northern Africa and with a set of sun photometer measurements located at Banizoumbou, Cinzana, Soroa, Mbour and Cape Verde. The vertical distribution of dust aerosol represented by extinction profiles is also analysed using CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) observations. The annual dust emission simulated by ALADIN over northern Africa is 878 Tg year-1. The Bodélé Depression appears to be the main area of dust emission in northern Africa, with an average estimate of about 21.6 Tg year-1. The simulated AOTs are in good agreement with satellite and sun photometer observations. The positions of the maxima of the modelled AOTs over northern Africa match the observed positions, and the ALADIN simulations satisfactorily reproduce the various dust events over the 2006-2010 period. The AOT climatology proposed in this paper provides a solid database of optical properties and consolidates the existing climatology over this region derived from satellites, the AERONET network and regional climate

  12. The paleo-ocean characteristics of the Taklimakan dust aerosol: high sulfate from primary sources and implication for climate modeling

    NASA Astrophysics Data System (ADS)

    Huang, K.; Zhuang, G.; Fu, J. S.; Dong, X.

    2017-12-01

    Multi-year monitoring of dust aerosol from the Taklimakan Desert has been conducted at one site in the hinterland of the desert, Tazhong and another site at the southern edge of the desert, Hotan. Compared to the other two important desert source regions of China, i.e. Gobi and Loess Plateau, the Taklimakan Desert is characterized of high calcium with a Ca/Al elemental ratio of around 1.50. The unique feature of the Taklimakan dust aerosol is its abundant sulfate. For instance, the mean concentration of sulfate over Tazhong reached as high as 34.7 and 48.8 ug/m3 during the spring of 2007 and 2008, respectively. During the dust storm events, the daily concentration of sulfate frequently exceeded 100 ug/m3. Sulfate showed strong correlations with the primary aerosol species such as Ca2+, Mg2+, Na+, Cl-, Al, Fe, Ti, etc. but weakly correlated with the secondary aerosol species such as NO3- and NH4+. The mass ratio of sulfate in the total suspended particles showed a relatively stable percentage of around 2.5% regardless of the intensity of the dust events. In addition, individual particle analysis using the scanning electron microscope (SEM) technique found that gypsum (CaSO4) particles could account for 11.1% of total number of particles as well as abundant Na2SO4 and NaCl particles. All the evidences above suggested the high sulfate observed in the Taklimakan Desert were largely attributed to primary sources but not formed via the traditional gas-to-particle formation pathway. As the Taklimakan Desert was speculated to be ocean 5-7 million years, the dried sea salts from the paleo-ocean should be the major source of the dust aerosol. Also, the dried salt lakes in the northwestern China may contribute to the high sulfate. Based on two different methods, the contribution of primary sources to sulfate over the Taklimakan Desert is estimated to be around 43% - 82%. This study implied that the cooling effect of the Taklimakan dust aerosol could be underestimated if the

  13. Atmosphere aerosol/dust composition over central Asia and western Siberia derived from snow/ice core records and calibrated with NASA remote sensing data

    NASA Astrophysics Data System (ADS)

    Aizen, V. B.; Aizen, E. M.; Joswiak, D. R.; Surazakov, A. B.; Takeuchi, N.

    2007-12-01

    The vast arid and semi-arid regions of central Asia, Mongolia, and Northern China are the world's second largest source of atmospheric mineral dust. In recent years, severe dust storms in Asia have intensified in frequency, duration, and areal coverage. However, limited spatial and temporal extent of aerosol measurements precludes definitive statements to be made regarding relationship between the Asian aerosol generation and climate. It has been well known that glaciers are the natural archives of environmental records related to past climate and aerosol generation. In our research, we utilized central Asian and western Siberia shallow ice-core records recovered from Altai, Tien Shan and Pamir mountain glaciers. Despite the fact that ice-core data may extend climate/aerosol records back in time, their sparse coverage is inadequate to document aerosol spatial distribution. The NASA products from Aura, Terra and Aqua satellite missions address this gap identifying aerosol sources, transport pathways, and area of deposition. The main objective of our research is to evaluate an affect of climate variability on dynamics of Asian aerosol loading to atmosphere and changes in aerosol transport pathways. Dust particle, major and rare earth element analysis from dust aerosols deposited and accumulated in Altai, Tien Shan and Pamir glaciers suggests that loess from Tajikistan, Afghanistan and north-western China are main sources of aerosol loading into the upper troposphere over the central Asia and western Siberia. At the same time, the soluble ionic component of the ice-cores, related to aerosol generated from evaporate deposits, demonstrated both anthropogenic and natural impacts on atmospheric chemistry over these regions. Large perturbations of Ca2+ derived from CaCO3- rich dust transported from Goby Desert to Altai and Tien Shan. Origin and pathway of the ice-core aerosol depositions for the last 10-years were identified through calibrating ice-core records with dust

  14. A Global Data Assimilation System for Atmospheric Aerosol

    NASA Technical Reports Server (NTRS)

    daSilva, Arlindo

    1999-01-01

    We will give an overview of an aerosol data assimilation system which combines advances in remote sensing of atmospheric aerosols, aerosol modeling and data assimilation methodology to produce high spatial and temporal resolution 3D aerosol fields. Initially, the Goddard Aerosol Assimilation System (GAAS) will assimilate TOMS, AVHRR and AERONET observations; later we will include MODIS and MISR. This data assimilation capability will allows us to integrate complementing aerosol observations from these platforms, enabling the development of an assimilated aerosol climatology as well as a global aerosol forecasting system in support of field campaigns. Furthermore, this system provides an interactive retrieval framework for each aerosol observing satellites, in particular TOMS and AVHRR. The Goddard Aerosol Assimilation System (GAAS) takes advantage of recent advances in constituent data assimilation at DAO, including flow dependent parameterizations of error covariances and the proper consideration of model bias. For its prognostic transport model, GAAS will utilize the Goddard Ozone, Chemistry, Aerosol, Radiation and Transport (GOCART) model developed at NASA/GSFC Codes 916 and 910.3. GOCART includes the Lin-Rood flux-form, semi-Langrangian transport model with parameterized aerosol chemistry and physical processes for absorbing (dust and black carbon) and non-absorbing aerosols (sulfate and organic carbon). Observations and model fields are combined using a constituent version of DAO's Physical-space Statistical Analysis System (PSAS), including its adaptive quality control system. In this talk we describe the main components of this assimilation system and present preliminary results obtained by assimilating TOMS data.

  15. Desert Dust Aerosol Air Mass Mapping in the Western Sahara, Using Particle Properties Derived from Space-Based Multi-Angle Imaging

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph; Petzold, Andreas; Wendisch, Manfred; Bierwirth, Eike; Dinter, Tilman; Esselborn, Michael; Fiebig, Marcus; Heese, Birgit; Knippertz, Peter; Mueller, Detlef; hide

    2008-01-01

    Coincident observations made over the Moroccan desert during the Sahara mineral dust experiment (SAMUM) 2006 field campaign are used both to validate aerosol amount and type retrieved from multi-angle imaging spectroradiometer (MISR) observations, and to place the suborbital aerosol measurements into the satellite s larger regional context. On three moderately dusty days during which coincident observations were made, MISR mid-visible aerosol optical thickness (AOT) agrees with field measurements point-by-point to within 0.05 0.1. This is about as well as can be expected given spatial sampling differences; the space-based observations capture AOT trends and variability over an extended region. The field data also validate MISR s ability to distinguish and to map aerosol air masses, from the combination of retrieved constraints on particle size, shape and single-scattering albedo. For the three study days, the satellite observations (1) highlight regional gradients in the mix of dust and background spherical particles, (2) identify a dust plume most likely part of a density flow and (3) show an aerosol air mass containing a higher proportion of small, spherical particles than the surroundings, that appears to be aerosol pollution transported from several thousand kilometres away.

  16. Ultraviolet dust aerosol properties as observed by MARCI

    NASA Astrophysics Data System (ADS)

    Wolff, Michael J.; Todd Clancy, R.; Goguen, Jay D.; Malin, Michael C.; Cantor, Bruce A.

    2010-07-01

    Observations by the Mars Color Imager (MARCI) on board the Mars Reconnaissance Orbiter (MRO) in two ultraviolet (UV, Bands 6 and 7; 258 nm, and 320 nm, respectively) and one visible (Band 1, 436 nm) channels of the 2007 planet encircling dust storm are combined with those made by the two Mars Exploration Rovers (MERs) to better characterize the single scattering albedo (ω0) of martian dust aerosols. Exploiting the low contrast of the surface in the UV (and blue) as well as the reduced importance of surface reflectance under very dusty conditions, we utilize the sampling of photometric angles by the MARCI cross-track geometry to synthesize an analog of the classical Emergence Phase Function (EPF). This so-called "pseudo-EPF", used in conjunction with the "ground-truth" measurements provided by the MERs, is able to effectively isolate the effects of the dust ω0. The motivation for this approach is the elimination of a significant portion of the type of uncertainty involved in many previous radiative transfer analyses. Furthermore, we produce a self-consistent set of complex refractive indices (m=n+ik) through our use of an explicit microphysical representation of the aerosol scattering properties. Because of uncertainty in the exact size of the dust particles during the epoch of the observations, we consider two effective particle radii (reff) to cover the range anticipated from the literature: 1.6 and 1.8 μm. The resulting set of model-data comparisons, ω0, and m are presented along with an assessment of potential sources of error and uncertainty. Analysis of the Band 1 results is limited to ω0 as a "proof-of-concept" for our approach through a comparison to contemporaneous CRISM EPF results at 440 nm. The derived ω0 are: assuming reff=1.6μm-0.619-0.626,0.648, and 0.765, for Bands 6, 7, and 1, respectively; for reff=1.8μm-0.625-0.635,0.653,0.769, for the same band order. For either reff case, the total estimated error is 0.022, 0.019, and 0.010, again for

  17. A review on the importance of metals and metalloids in atmospheric dust and aerosol from mining operations.

    PubMed

    Csavina, Janae; Field, Jason; Taylor, Mark P; Gao, Song; Landázuri, Andrea; Betterton, Eric A; Sáez, A Eduardo

    2012-09-01

    Contaminants can be transported rapidly and over relatively long distances by atmospheric dust and aerosol relative to other media such as water, soil and biota; yet few studies have explicitly evaluated the environmental implications of this pathway, making it a fundamental but understudied transport mechanism. Although there are numerous natural and anthropogenic activities that can increase dust and aerosol emissions and contaminant levels in the environment, mining operations are notable with respect to the quantity of particulates generated, the global extent of area impacted, and the toxicity of contaminants associated with the emissions. Here we review (i) the environmental fate and transport of metals and metalloids in dust and aerosol from mining operations, (ii) current methodologies used to assess contaminant concentrations and particulate emissions, and (iii) the potential health and environmental risks associated with airborne contaminants from mining operations. The review evaluates future research priorities based on the available literature and suggest that there is a particular need to measure and understand the generation, fate and transport of airborne particulates from mining operations, specifically the finer particle fraction. More generally, our findings suggest that mining operations play an important but underappreciated role in the generation of contaminated atmospheric dust and aerosol and the transport of metal and metalloid contaminants, and highlight the need for further research in this area. The role of mining activities in the fate and transport of environmental contaminants may become increasingly important in the coming decades, as climate change and land use are projected to intensify, both of which can substantially increase the potential for dust emissions and transport. Copyright © 2012 Elsevier B.V. All rights reserved.

  18. A Review on the Importance of Metals and Metalloids in Atmospheric Dust and Aerosol from Mining Operations

    PubMed Central

    Csavina, Janae; Field, Jason; Taylor, Mark P.; Gao, Song; Landázuri, Andrea; Betterton, Eric A.; Sáez, A. Eduardo

    2012-01-01

    Contaminants can be transported rapidly and over relatively long distances by atmospheric dust and aerosol relative to other media such as water, soil and biota; yet few studies have explicitly evaluated the environmental implications of this pathway, making it a fundamental but understudied transport mechanism. Although there are numerous natural and anthropogenic activities that can increase dust and aerosol emissions and contaminant levels in the environment, mining operations are notable with respect to the quantity of particulates generated, the global extent of area impacted, and the toxicity of contaminants associated with the emissions. Here we review (i) the environmental fate and transport of metals and metalloids in dust and aerosol from mining operations, (ii) current methodologies used to assess contaminant concentrations and particulate emissions, and (iii) the potential health and environmental risks associated with airborne contaminants from mining operations. The review evaluates future research priorities based on the available literature and suggest that there is a particular need to measure and understand the generation, fate and transport of airborne particulates from mining operations, specifically the finer particle fraction. More generally, our findings suggest that mining operations play an important but underappreciated role in the generation of contaminated atmospheric dust and aerosol and the transport of metal and metalloid contaminants, and highlight the need for further research in this area. The role of mining activities in the fate and transport of environmental contaminants may become increasingly important in the coming decades, as climate change and land use are projected to intensify, both of which can substantially increase the potential for dust emissions and transport. PMID:22766428

  19. Dust feed mechanism

    DOEpatents

    Milliman, Edward M.

    1984-01-01

    The invention is a dust feed device for delivery of a uniform supply of dust for long periods of time to an aerosolizing means for production of a dust suspension. The device utilizes at least two tandem containers having spiral brushes within the containers which transport the dust from a supply to the aerosolizer means.

  20. The implementation of NEMS GFS Aerosol Component (NGAC) Version 1.0 for global dust forecasting at NOAA/NCEP

    PubMed Central

    Lu, Cheng-Hsuan; da Silva, Arlindo; Wang, Jun; Moorthi, Shrinivas; Chin, Mian; Colarco, Peter; Tang, Youhua; Bhattacharjee, Partha S.; Chen, Shen-Po; Chuang, Hui-Ya; Juang, Hann-Ming Henry; McQueen, Jeffery; Iredell, Mark

    2018-01-01

    The NOAA National Centers for Environmental Prediction (NCEP) implemented NEMS GFS Aerosol Component (NGAC) for global dust forecasting in collaboration with NASA Goddard Space Flight Center (GSFC). NGAC Version 1.0 has been providing 5 day dust forecasts at 1°×1° resolution on a global scale, once per day at 00:00 Coordinated Universal Time (UTC), since September 2012. This is the first global system capable of interactive atmosphere aerosol forecasting at NCEP. The implementation of NGAC V1.0 reflects an effective and efficient transitioning of NASA research advances to NCEP operations, paving the way for NCEP to provide global aerosol products serving a wide range of stakeholders as well as to allow the effects of aerosols on weather forecasts and climate prediction to be considered. PMID:29652411

  1. The implementation of NEMS GFS Aerosol Component (NGAC) Version 1.0 for global dust forecasting at NOAA/NCEP.

    PubMed

    Lu, Cheng-Hsuan; da Silva, Arlindo; Wang, Jun; Moorthi, Shrinivas; Chin, Mian; Colarco, Peter; Tang, Youhua; Bhattacharjee, Partha S; Chen, Shen-Po; Chuang, Hui-Ya; Juang, Hann-Ming Henry; McQueen, Jeffery; Iredell, Mark

    2016-01-01

    The NOAA National Centers for Environmental Prediction (NCEP) implemented NEMS GFS Aerosol Component (NGAC) for global dust forecasting in collaboration with NASA Goddard Space Flight Center (GSFC). NGAC Version 1.0 has been providing 5 day dust forecasts at 1°×1° resolution on a global scale, once per day at 00:00 Coordinated Universal Time (UTC), since September 2012. This is the first global system capable of interactive atmosphere aerosol forecasting at NCEP. The implementation of NGAC V1.0 reflects an effective and efficient transitioning of NASA research advances to NCEP operations, paving the way for NCEP to provide global aerosol products serving a wide range of stakeholders as well as to allow the effects of aerosols on weather forecasts and climate prediction to be considered.

  2. Tropical Atlantic Dust and Smoke Aerosol Variations Related to the Madden-Julian Oscillation in MODIS and MISR Observations

    NASA Technical Reports Server (NTRS)

    Guo, Yanjuan; Tian, Baijun; Kahn, Ralph A.; Kalashnikova, Olga; Wong, Sun; Waliser, Duane E.

    2013-01-01

    In this study, Moderate Resolution Imaging Spectroradiometer (MODIS) fine mode fraction and Multi-angle Imaging SpectroRadiometer (MISR) nonspherical fraction data are used to derive dust and smoke aerosol optical thickness (T(sub dust) and T(sub smoke)) over the tropical Atlantic in a complementary way: due to its wider swath, MODIS has 3-4 times greater sampling than MISR, but MISR dust discrimination is based on particle shape retrievals, whereas an empirical scheme is used for MODIS. MODIS and MISR show very similar dust and smoke winter climatologies. T(sub dust) is the dominant aerosol component over the tropical Atlantic, accounting for 40-70 percent of the total aerosol optical thickness (AOT), whereas T(sub smoke) is significantly smaller than T(sub dust). The consistency and high correlation between these climatologies and their daily variations lends confidence to their use for investigating the relative dust and smoke contributions to the total AOT variation associated with the Madden-Julian Oscillation (MJO). The temporal evolution and spatial patterns of the tdus anomalies associated with the MJO are consistent between MODIS and MISR: the magnitude of MJO-realted T(sub dust) anomalies is comparable to or even larger than that of the total T, while the T(sub smoke) anomaly represents about 15 percent compared to the total, which is quite different from their relative magnitudes to the total T on the climatological time scale. This suggests that dust and smoke are not influenced by the MJO in the same way. Based on correlation analysis, dust is strongly influenced by the MJO-modulated trade wind and precipitation anomalies, and can last as long as one MJO phase, whereas smoke is less affected.

  3. Enhanced Surface Warming and Accelerated Snow Melt in the Himalayas and Tibetan Plateau Induced by Absorbing Aerosols

    NASA Technical Reports Server (NTRS)

    Lau, William K.; Kim, Maeng-Ki; Kim, Kyu-Myong; Lee, Woo-Seop

    2010-01-01

    Numerical experiments with the NASA finite-volume general circulation model show that heating of the atmosphere by dust and black carbon can lead to widespread enhanced warming over the Tibetan Plateau (TP) and accelerated snow melt in the western TP and Himalayas. During the boreal spring, a thick aerosol layer, composed mainly of dust transported from adjacent deserts and black carbon from local emissions, builds up over the Indo-Gangetic Plain, against the foothills of the Himalaya and the TP. The aerosol layer, which extends from the surface to high elevation (approx.5 km), heats the mid-troposphere by absorbing solar radiation. The heating produces an atmospheric dynamical feedback the so-called elevated-heat-pump (EHP) effect, which increases moisture, cloudiness, and deep convection over northern India, as well as enhancing the rate of snow melt in the Himalayas and TP. The accelerated melting of snow is mostly confined to the western TP, first slowly in early April and then rapidly from early to mid-May. The snow cover remains reduced from mid-May through early June. The accelerated snow melt is accompanied by similar phases of enhanced warming of the atmosphere-land system of the TP, with the atmospheric warming leading the surface warming by several days. Surface energy balance analysis shows that the short-wave and long-wave surface radiative fluxes strongly offset each other, and are largely regulated by the changes in cloudiness and moisture over the TP. The slow melting phase in April is initiated by an effective transfer of sensible heat from a warmer atmosphere to land. The rapid melting phase in May is due to an evaporation-snow-land feedback coupled to an increase in atmospheric moisture over the TP induced by the EHP effect.

  4. Saharan dust, convective lofting, aerosol enhancement zones, and potential impacts on ice nucleation in the tropical upper troposphere

    NASA Astrophysics Data System (ADS)

    Twohy, C. H.; Anderson, B. E.; Ferrare, R. A.; Sauter, K. E.; L'Ecuyer, T. S.; van den Heever, S. C.; Heymsfield, A. J.; Ismail, S.; Diskin, G. S.

    2017-08-01

    Dry aerosol size distributions and scattering coefficients were measured on 10 flights in 32 clear-air regions adjacent to tropical storm anvils over the eastern Atlantic Ocean. Aerosol properties in these regions were compared with those from background air in the upper troposphere at least 40 km from clouds. Median values for aerosol scattering coefficient and particle number concentration >0.3 μm diameter were higher at the anvil edges than in background air, showing that convective clouds loft particles from the lower troposphere to the upper troposphere. These differences are statistically significant. The aerosol enhancement zones extended 10-15 km horizontally and 0.25 km vertically below anvil cloud edges but were not due to hygroscopic growth since particles were measured under dry conditions. Number concentrations of particles >0.3 μm diameter were enhanced more for the cases where Saharan dust layers were identified below the clouds with airborne lidar. Median number concentrations in this size range increased from 100 l-1 in background air to 400 l-1 adjacent to cloud edges with dust below, with larger enhancements for stronger storm systems. Integration with satellite cloud frequency data indicates that this transfer of large particles from low to high altitudes by convection has little impact on dust concentrations within the Saharan Air Layer itself. However, it can lead to substantial enhancement in large dust particles and, therefore, heterogeneous ice nuclei in the upper troposphere over the Atlantic. This may induce a cloud/aerosol feedback effect that could impact cloud properties in the region and downwind.

  5. Spatio-temporal interaction between absorbing aerosols and temperature: Correlation and causality based approach

    NASA Astrophysics Data System (ADS)

    Dave, P.; Bhushan, M.; Venkataraman, C.

    2016-12-01

    Indian subcontinent, in particular, the Indo-gangetic plain (IGP) has witnessed large temperature anomalies (Ratnam et al., 2016) along with high emission of absorbing aerosols (AA) (Gazala, et al., 2005). The anomalous high temperature observed over this region may bear a relationship with high AA emissions. Different studies have been conducted to understand AA and temperature relationships (Turco et al., 1983; Hansen et al., 1997, 2005; Seinfeld 2008; Ramanathan et al. 2010b; Ban-Weiss et al., 2012). It was found that when the AA was injected in the lower- mid troposphere the surface air temperature increases while injection of AA at higher troposphere-lower stratosphere surface temperature decreases. These studies used simulation based results to establish link between AA and temperature (Hansen et al., 1997, 2005; Ban-Weiss et al., 2012). The current work focuses on identifying the causal influence of AA on temperature using observational and re-analysis data over Indian subcontinent using cross correlation (CCs) and Granger causality (GC) (Granger, 1969). Aerosol index (AI) from TOMS-OMI was used as index for AA while ERA-interim reanalysis data was used for temperature at varying altitude. Period of study was March-April-May-June (MAMJ) for years 1979-2015. CCs were calculated for all the atmospheric layers. In each layer nearby and distant pixels (>500 kms) with high CCs were identified using clustering technique. It was found that that AI and Temperature shows statistically significant cross-correlations for co-located and distant pixels and more prominently over IGP. The CCs fades away with higher altitudes. CCs analysis was followed by GC analysis to identify the lag over which AI can influence the Temperature. GC also supported the findings of CCs analysis. It is an early attempt to link persisting large temperature anomalies with absorbing aerosols and may help in identifying the role of absorbing aerosol in causing heat waves.

  6. The Continuous Monitoring of Desert Dust using an Infrared-based Dust Detection and Retrieval Method

    NASA Technical Reports Server (NTRS)

    Duda, David P.; Minnis, Patrick; Trepte, Qing; Sun-Mack, Sunny

    2006-01-01

    Airborne dust and sand are significant aerosol sources that can impact the atmospheric and surface radiation budgets. Because airborne dust affects visibility and air quality, it is desirable to monitor the location and concentrations of this aerosol for transportation and public health. Although aerosol retrievals have been derived for many years using visible and near-infrared reflectance measurements from satellites, the detection and quantification of dust from these channels is problematic over bright surfaces, or when dust concentrations are large. In addition, aerosol retrievals from polar orbiting satellites lack the ability to monitor the progression and sources of dust storms. As a complement to current aerosol dust retrieval algorithms, multi-spectral thermal infrared (8-12 micron) data from the Moderate Resolution Imaging Spectroradiometer (MODIS) and the Meteosat-8 Spinning Enhanced Visible and Infrared Imager (SEVIRI) are used in the development of a prototype dust detection method and dust property retrieval that can monitor the progress of Saharan dust fields continuously, both night and day. The dust detection method is incorporated into the processing of CERES (Clouds and the Earth s Radiant Energy System) aerosol retrievals to produce dust property retrievals. Both MODIS (from Terra and Aqua) and SEVERI data are used to develop the method.

  7. A multi-satellite analysis of the direct radiative effects of absorbing aerosols above clouds

    NASA Astrophysics Data System (ADS)

    Chang, Y. Y.; Christopher, S. A.

    2015-12-01

    Radiative effects of absorbing aerosols above liquid water clouds in the southeast Atlantic as a function of fire sources are investigated using A-Train data coupled with the Visible Infrared Imaging Radiometer Suite (VIIRS) onboard Suomi National Polar-orbiting Partnership (Suomi NPP). Both the VIIRS Active Fire product and the Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) Thermal Anomalies product (MYD14) are used to identify the biomass burning fire origin in southern Africa. The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) are used to assess the aerosol type, aerosol altitude, and cloud altitude. We use back trajectory information, wind data, and the Fire Locating and Modeling of Burning Emissions (FLAMBE) product to infer the transportation of aerosols from the fire source to the CALIOP swath in the southeast Atlantic during austral winter.

  8. Laboratory Measurements of Mass Specific Absorption Spectra for Suites of Black Carbon-like, Biomass Burning and Mineral Dust Aerosols

    NASA Astrophysics Data System (ADS)

    Radney, J.; Zangmeister, C.

    2017-12-01

    Light-absorbing atmospheric aerosols can be grouped into three categories: black carbon (BC), brown carbon (BrC) or mineral dust (MD). In many cases, the absorption of these species is best quantified using a mass-specific absorption cross section (MAC) since the particles are in the Rayleigh regime (BC) or optically thin (BrC and MD); notably, MAC values are both traceable to the SI and transferrable between photoacoustic spectroscopy and filter-based absorption measurements. Here, we present laboratory measurements of MAC for all three light-absorbing aerosol classes. Particles were size- and mass-selected using a differential mobility analyzer and aerosol particle mass analyzer, respectively, with absorption coefficients (αabs) and number concentrations (N) being measured by a broadband photoacoustic spectrometer and condensation particle counter, respectively. This suite of instrumentation allows for direct quantification of MAC from the measured parameters (MAC = αabs/Nmp). Further, the measurements contained > 8 data points spanning λ = 405 nm to 840 nm allowing for spectral curvatures (i.e. the Absorption Angstrom Exponent or AAE) to be fit from many data points versus the more common 2-point interpolations. For the carbonaceous, BC-like aerosols - five samples generated from flames, spark discharge soot (i.e. fullerene soot), graphene, reduced graphene oxide (rGO), and fullerene (C60) - we found: 1) measured MAC ranged between 2.4 m2 g-1 and 8.6 m2 g-1 at λ = 550 nm, 2) most AAEs ranged between 0.5 and 1.3; C60 AAE was 7.5 ± 0.9 and 3) MAC spectra were dependent on fuel type and formation conditions. For BrC particles generated from smoldering combustion of 3 hardwood (Oak, Hickory and Mesquite) and 3 softwood species (Western redcedar, Blue spruce and Baldcypress), we found: 1) median MAC values ranged from 1.4 x 10-2 m2 g-1 to 7.9 x 10-2 m2 g-1 at λ = 550 nm, 2) AAE values ranged between 3.5 and 6.2, and 3) Oak, Western redcedar and Blue spruce

  9. Sensitivity of Multiangle Imaging to the Optical and Microphysical Properties of Biomass Burning Aerosols

    NASA Technical Reports Server (NTRS)

    Chen, Wei-Ting; Kahn, Ralph A.; Nelson, David; Yau, Kevin; Seinfeld, John H.

    2008-01-01

    The treatment of biomass burning (BB) carbonaceous particles in the Multiangle Imaging SpectroRadiometer (MISR) Standard Aerosol Retrieval Algorithm is assessed, and algorithm refinements are suggested, based on a theoretical sensitivity analysis and comparisons with near-coincident AERONET measurements at representative BB sites. Over the natural ranges of BB aerosol microphysical and optical properties observed in past field campaigns, patterns of retrieved Aerosol Optical Depth (AOD), particle size, and single scattering albedo (SSA) are evaluated. On the basis of the theoretical analysis, assuming total column AOD of 0.2, over a dark, uniform surface, MISR can distinguish two to three groups in each of size and SSA, except when the assumed atmospheric particles are significantly absorbing (mid-visible SSA approx.0.84), or of medium sizes (mean radius approx.0.13 pin); sensitivity to absorbing, medium-large size particles increases considerably when the assumed column AOD is raised to 0.5. MISR Research Aerosol Retrievals confirm the theoretical results, based on coincident AERONET inversions under BB-dominated conditions. When BB is externally mixed with dust in the atmosphere, dust optical model and surface reflection uncertainties, along with spatial variability, contribute to differences between the Research Retrievals and AERONET. These results suggest specific refinements to the MISR Standard Aerosol Algorithm complement of component particles and mixtures. They also highlight the importance for satellite aerosol retrievals of surface reflectance characterization, with accuracies that can be difficult to achieve with coupled surface-aerosol algorithms in some higher AOD situations.

  10. The Regional Environmental Impacts of Atmospheric Aerosols over Egypt

    NASA Astrophysics Data System (ADS)

    Zakey, Ashraf; Ibrahim, Alaa

    2015-04-01

    Identifying the origin (natural versus anthropogenic) and the dynamics of aerosols over Egypt at varying temporal and spatial scales provide valuable knowledge on the regional climate impacts of aerosols and their ultimate connections to the Earth's regional climate system at the MENA region. At regional scale, Egypt is exposed to air pollution with levels exceeding typical air-quality standards. This is particularly true for the Nile Delta region, being at the crossroads of different aerosol species originating from local urban-industrial and biomass-burning activities, regional dust sources, and European pollution from the north. The Environmental Climate Model (EnvClimA) is used to investigate both of the biogenic and anthropogenic aerosols over Egypt. The dominant natural aerosols over Egypt are due to the sand and dust storms, which frequently occur during the transitional seasons (spring and autumn). In winter, the maximum frequency reaches 2 to 3 per day in the north, which decreases gradually southward with a frequency of 0.5-1 per day. Monitoring one of the most basic aerosol parameters, the aerosol optical depth (AOD), is a main experimental and modeling task in aerosol studies. We used the aerosol optical depth to quantify the amount and variability of aerosol loading in the atmospheric column over a certain areas. The aerosols optical depth from the model is higher in spring season due to the impacts of dust activity over Egypt as results of the westerly wind, which carries more dust particles from the Libyan Desert. The model result shows that the mass load of fine aerosols has a longer life-time than the coarse aerosols. In autumn season, the modelled aerosol optical depth tends to increase due to the biomass burning in the delta of Egypt. Natural aerosol from the model tends to scatter the solar radiation while most of the anthropogenic aerosols tend to absorb the longwave solar radiation. The overall results indicate that the AOD is lowest in winter

  11. Aerosol Impacts on California Winter Clouds and Precipitation during CalWater 2011: Local Pollution versus Long-Range Transported Dust

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Fan, Jiwen; Leung, Lai-Yung R.; DeMott, Paul J.

    2014-01-03

    Mineral dust aerosols often observed over California in winter and spring, associated with long-range transport from Asia and Sahara, have been linked to enhanced precipitation based on observations. Local anthropogenic pollution, on the other hand, was shown in previous observational and modeling studies to reduce precipitation. Here we incorporate recent developments in ice nucleation parameterizations to link aerosols with ice crystal formation in a spectral-bin cloud microphysical model coupled with the Weather Research and Forecasting (WRF) model, to examine the relative and combined impacts of dust and local pollution particles on cloud properties and precipitation type and intensity. Simulations aremore » carried out for two cloud cases with contrasting meteorology and cloud dynamics that occurred on February 16 (FEB16) and March 02 (MAR02) from the CalWater 2011 field campaign. In both cases, observations show the presence of dust and biological particles in a relative pristine environment. The simulated cloud microphysical properties and precipitation show reasonable agreement with aircraft and surface measurements. Model sensitivity experiments indicate that in the pristine environment, the dust and biological aerosol layers increase the accumulated precipitation by 10-20% from the Central Valley to the Sierra Nevada Mountains for both FEB16 and MAR02 due to a ~40% increase in snow formation, validating the observational hypothesis. Model results show that local pollution increases precipitation over the windward slope of the mountains by few percent due to increased snow formation when dust is present but reduces precipitation by 5-8% if dust is removed on FEB16. The effects of local pollution on cloud microphysics and precipitation strongly depend on meteorology including the strength of the Sierra Barrier Jet, and cloud dynamics. This study further underscores the importance of the interactions between local pollution, dust, and environmental

  12. Impact of absorbing aerosol deposition on snow albedo reduction over the southern Tibetan plateau based on satellite observations

    NASA Astrophysics Data System (ADS)

    Lee, Wei-Liang; Liou, K. N.; He, Cenlin; Liang, Hsin-Chien; Wang, Tai-Chi; Li, Qinbin; Liu, Zhenxin; Yue, Qing

    2017-08-01

    We investigate the snow albedo variation in spring over the southern Tibetan Plateau induced by the deposition of light-absorbing aerosols using remote sensing data from moderate resolution imaging spectroradiometer (MODIS) aboard Terra satellite during 2001-2012. We have selected pixels with 100 % snow cover for the entire period in March and April to avoid albedo contamination by other types of land surfaces. A model simulation using GEOS-Chem shows that aerosol optical depth (AOD) is a good indicator for black carbon and dust deposition on snow over the southern Tibetan Plateau. The monthly means of satellite-retrieved land surface temperature (LST) and AOD over 100 % snow-covered pixels during the 12 years are used in multiple linear regression analysis to derive the empirical relationship between snow albedo and these variables. Along with the LST effect, AOD is shown to be an important factor contributing to snow albedo reduction. We illustrate through statistical analysis that a 1-K increase in LST and a 0.1 increase in AOD indicate decreases in snow albedo by 0.75 and 2.1 % in the southern Tibetan Plateau, corresponding to local shortwave radiative forcing of 1.5 and 4.2 W m-2, respectively.

  13. Light scattering by dust and anthropogenic aerosol at a remote site in the Negev desert, Israel

    NASA Astrophysics Data System (ADS)

    Andreae, Tracey W.; Andreae, Meinrat O.; Ichoku, Charles; Maenhaut, Willy; Cafmeyer, Jan; Karnieli, Arnon; Orlovsky, Leah

    2002-01-01

    We investigated aerosol optical properties, mass concentration, and chemical composition over a 2 year period at a remote site in the Negev desert, Israel (Sde Boker, 30° 51'N, 34° 47'E, 470 m above sea level). Light-scattering measurements were made at three wavelengths (450, 550, and 700 nm), using an integrating nephelometer, and included the separate determination of the backscatter fraction. Aerosol coarse and fine fractions were collected with stacked filter units; mass concentrations were determined by weighing, and the chemical composition by proton-induced X-ray emission and instrumental neutron activation analysis. The total scattering coefficient at 550 nm showed a median of 66.7 Mm-1(mean value 75.2 Mm-1, standard deviation 41.7 Mm-1) typical of moderately polluted continental air masses. Values of 1000 Mm-1and higher were encountered during severe dust storm events. During the study period, 31 such dust events were detected. In addition to high scattering levels, they were characterized by a sharp drop in the Ångström coefficient (i.e., the spectral dispersion of the light scattering) to values near zero. Mass-scattering efficiencies were obtained by a multivariate regression of the scattering coefficients on dust, sulfate, and residual components. An analysis of the contributions of these components to the total scattering observed showed that anthropogenic aerosol accounted for about 70% of scattering. The rest was dominated by the effect of the large dust events mentioned above and of small dust episodes typically occurring during midafternoon.

  14. Deciphering the Role of Desert Dust in the Climate Puzzle: The Mediterranean Israeli Dust Experiment (MEIDEX)

    NASA Technical Reports Server (NTRS)

    Levin, Zev; Joseph, Joachim; Mekler, Yuri; Israelevich, Peter; Ganor, Eli; Hilsenrath, Ernest; Janz, Scott

    2002-01-01

    Numerous studies have shown that aerosol particles may be one of the primary agents that can offset the climate warming induced by the increase in the amount of atmospheric greenhouse gases. Desert aerosols are probably the most abundant and massive type of aerosol particles that are present in the atmosphere worldwide. These aerosols are carried over large distances and have various global impacts. They interact with clouds, impact the efficiency of their rain production and change their optical properties. They constitute one of the primary sources of minerals for oceanic life and influence the health of coral reefs. They have direct effects on human health, especially by inducing breathing difficulties in children. It was lately discovered that desert particles carry pathogens from the Sahara desert over the Atlantic Ocean, a fact that may explain the migration of certain types of diseases. Aerosols not only absorb solar radiation but also scatter it, so that their climatic effect is influenced not only by their physical properties and height distribution but also by the reflectivity of the underlying surface. This latter property changes greatly over land and is low over ocean surfaces. Aerosol plumes are emitted from discrete, sporadic sources in the desert areas of the world and are transported worldwide by the atmosphere's wind systems. For example, Saharan dust reaches Mexico City, Florida, Ireland, Switzerland and the Mediterranean region, while Asian dust reaches Alaska, Hawaii and the continental United States. This means that in order to assess its global effects, one must observe dust from space. The Space Shuttle is a unique platform, because it flies over the major deserts of our planet, enabling measurements and remote sensing of the aerosols as they travel from source to sink regions. Such efforts must always be accompanied by in-situ data for validation and calibration, with direct sampling of the airborne particles. MEIDEX is a joint project of

  15. Satellite-Based Assessment of Possible Dust Aerosols Semi-Direct Effect on Cloud Water Path over East Asia

    NASA Technical Reports Server (NTRS)

    Huang, Jianping; Lin, Bing; Minnis, Patrick; Wang, Tainhe; Wang, Xin; Hu, Yongxiang; Yi, Yuhong; Ayers, J. Kirk

    2006-01-01

    The semi-direct effects of dust aerosols are analyzed over eastern Asia using 2 years (June 2002 to June 2004) of data from the Clouds and the Earth s Radiant Energy System (CERES) scanning radiometer and MODerate Resolution Imaging Spectroradiometer (MODIS) on the Aqua satellite, and 18 years (1984 to 2001) of International Satellite Cloud Climatology Project (ISCCP) data. The results show that the water path of dust-contaminated clouds is considerably smaller than that of dust-free clouds. The mean ice water path (IWP) and liquid water path (LWP) of dusty clouds are less than their dust-free counterparts by 23.7% and 49.8%, respectively. The long-term statistical relationship derived from ISCCP also confirms that there is significant negative correlation between dust storm index and ISCCP cloud water path. These results suggest that dust aerosols warm clouds, increase the evaporation of cloud droplets and further reduce cloud water path, the so-called semi-direct effect. The semi-direct effect may play a role in cloud development over arid and semi-arid areas of East Asia and contribute to the reduction of precipitation.

  16. A study of long-term trends in mineral dust aerosol distributions in Asia using a general circulation model

    NASA Astrophysics Data System (ADS)

    Mukai, Makiko; Nakajima, Teruyuki; Takemura, Toshihiko

    2004-10-01

    Dust events have been observed in Japan with high frequency since 2000. On the other hand, the frequency of dust storms is said to have decreased in the desert regions of China since about the middle of the 1970s. This study simulates dust storms and transportation of mineral dust aerosols in the east Asia region from 1981 to 2001 using an aerosol transport model, Spectral Radiation-Transport Model for Aerosol Species (SPRINTARS), implemented in the Center for Climate System Research/National Institute for Environmental Studies atmospheric global circulation model, in order to investigate the main factors that control a dust event and its long-term variation. The model was forced to simulate a real atmospheric condition by a nudging technique using European Centre for Medium-Range Weather Forecasts reanalysis data on wind velocities, temperature, specific humidity, soil wetness, and snow depth. From a comparison between the long-term change in the dust emission and model parameters, it is found that the wind speed near the surface level had a significant influence on the dust emission, and snow is also an important factor in the early spring dust emission. The simulated results suggested that dust emissions from northeast China have a great impact on dust mass concentration in downwind regions, such as the cities of northeastern China, Korea, and Japan. When the frequency of dust events was high in Japan, a low-pressure system tended to develop over the northeast China region that caused strong winds. From 2000 to 2001 the simulated dust emission flux decreased in the Taklimakan desert and the northwestern part of China, while it increased in the Gobi desert and the northeastern part of China. Consequently, dust particles seem to be transported more from the latter region by prevailing westerlies in the springtime to downwind areas as actually observed. In spite of the similarity, however, there is still a large disagreement between observed and simulated dust

  17. The Implementation of NEMS GFS Aerosol Component (NGAC) Version 1.0 for Global Dust Forecasting at NOAA NCEP

    NASA Technical Reports Server (NTRS)

    Lu, Cheng-Hsuan; Da Silva, Arlindo M.; Wang, Jun; Moorthi, Shrinivas; Chin, Mian; Colarco, Peter; Tang, Youhua; Bhattacharjee, Partha S.; Chen, Shen-Po; Chuang, Hui-Ya; hide

    2016-01-01

    The NOAA National Centers for Environmental Prediction (NCEP) implemented the NOAA Environmental Modeling System (NEMS) Global Forecast System (GFS) Aerosol Component (NGAC) for global dust forecasting in collaboration with NASA Goddard Space Flight Center (GSFC). NGAC Version 1.0 has been providing 5-day dust forecasts at 1deg x 1deg resolution on a global scale, once per day at 00:00 Coordinated Universal Time (UTC), since September 2012. This is the first global system capable of interactive atmosphere aerosol forecasting at NCEP. The implementation of NGAC V1.0 reflects an effective and efficient transitioning of NASA research advances to NCEP operations, paving the way for NCEP to provide global aerosol products serving a wide range of stakeholders, as well as to allow the effects of aerosols on weather forecasts and climate prediction to be considered.

  18. Linking Barbados Mineral Dust Aerosols to North African Sources Using Elemental Composition and Radiogenic Sr, Nd, and Pb Isotope Signatures

    NASA Astrophysics Data System (ADS)

    Bozlaker, Ayse; Prospero, Joseph M.; Price, Jim; Chellam, Shankararaman

    2018-01-01

    Large quantities of African dust are carried across the Atlantic to the Caribbean Basin and southern United States where it plays an important role in the biogeochemistry of soils and waters and in air quality. Dusts' elemental and isotopic composition was comprehensively characterized in Barbados during the summers of 2013 and 2014, the season of maximum dust transport. Although total suspended insoluble particulate matter (TSIP) mass concentrations varied significantly daily and between the two summers, the abundances (μg element/g TSIP) of 50 elements during "high-dust days" (HDD) were similar. Aerosols were regularly enriched in Na, Cu, Zn, As, Se, Mo, Cd, Sn, Sb, and W relative to the upper continental crust. Enrichment of these elements, many of which are anthropogenically emitted, was significantly reduced during HDD, attributed to mixing and dilution with desert dust over source regions. Generally, Ti/Al, Si/Al, Ca/Al, Ti/Fe, Si/Fe, and Ca/Fe ratios during HDD differed from their respective values in hypothesized North African source regions. Nd isotope composition was relatively invariant for "low-dust days" (LDD) and HDD. In contrast, HDD-aerosols were more radiogenic exhibiting higher 87Sr/86Sr, 206Pb/204Pb, 207Pb/204Pb, and 208Pb/204Pb ratios compared to LDD. Generally, Barbados aerosols' composition ranged within narrow limits and was much more homogeneous than that of hypothesized African source soils. Our results suggest that summertime Barbados aerosols are dominated by a mixture of particles originating from sources in the Sahara-Sahel regions. The Bodélé Depression, long suspected as a major source, appears to be an insignificant contributor of summertime western Atlantic dust.

  19. Assimilation of MODIS Dark Target and Deep Blue Observations in the Dust Aerosol Component of NMMB-MONARCH version 1.0

    NASA Technical Reports Server (NTRS)

    Di Tomaso, Enza; Schutgens, Nick A. J.; Jorba, Oriol; Perez Garcia-Pando, Carlos

    2017-01-01

    A data assimilation capability has been built for the NMMB-MONARCH chemical weather prediction system, with a focus on mineral dust, a prominent type of aerosol. An ensemble-based Kalman filter technique (namely the local ensemble transform Kalman filter - LETKF) has been utilized to optimally combine model background and satellite retrievals. Our implementation of the ensemble is based on known uncertainties in the physical parametrizations of the dust emission scheme. Experiments showed that MODIS AOD retrievals using the Dark Target algorithm can help NMMB-MONARCH to better characterize atmospheric dust. This is particularly true for the analysis of the dust outflow in the Sahel region and over the African Atlantic coast. The assimilation of MODIS AOD retrievals based on the Deep Blue algorithm has a further positive impact in the analysis downwind from the strongest dust sources of the Sahara and in the Arabian Peninsula. An analysis-initialized forecast performs better (lower forecast error and higher correlation with observations) than a standard forecast, with the exception of underestimating dust in the long-range Atlantic transport and degradation of the temporal evolution of dust in some regions after day 1. Particularly relevant is the improved forecast over the Sahara throughout the forecast range thanks to the assimilation of Deep Blue retrievals over areas not easily covered by other observational datasets.The present study on mineral dust is a first step towards data assimilation with a complete aerosol prediction system that includes multiple aerosol species.

  20. Assimilation of MODIS Dark Target and Deep Blue observations in the dust aerosol component of NMMB-MONARCH version 1.0

    NASA Astrophysics Data System (ADS)

    Di Tomaso, Enza; Schutgens, Nick A. J.; Jorba, Oriol; Pérez García-Pando, Carlos

    2017-03-01

    A data assimilation capability has been built for the NMMB-MONARCH chemical weather prediction system, with a focus on mineral dust, a prominent type of aerosol. An ensemble-based Kalman filter technique (namely the local ensemble transform Kalman filter - LETKF) has been utilized to optimally combine model background and satellite retrievals. Our implementation of the ensemble is based on known uncertainties in the physical parametrizations of the dust emission scheme. Experiments showed that MODIS AOD retrievals using the Dark Target algorithm can help NMMB-MONARCH to better characterize atmospheric dust. This is particularly true for the analysis of the dust outflow in the Sahel region and over the African Atlantic coast. The assimilation of MODIS AOD retrievals based on the Deep Blue algorithm has a further positive impact in the analysis downwind from the strongest dust sources of the Sahara and in the Arabian Peninsula. An analysis-initialized forecast performs better (lower forecast error and higher correlation with observations) than a standard forecast, with the exception of underestimating dust in the long-range Atlantic transport and degradation of the temporal evolution of dust in some regions after day 1. Particularly relevant is the improved forecast over the Sahara throughout the forecast range thanks to the assimilation of Deep Blue retrievals over areas not easily covered by other observational datasets. The present study on mineral dust is a first step towards data assimilation with a complete aerosol prediction system that includes multiple aerosol species.

  1. Spectral Absorption Properties of Atmospheric Aerosols

    NASA Technical Reports Server (NTRS)

    Bergstrom, R. W.; Pilewskie, P.; Russell, P. B.; Redemann, J.; Bond, T. C.; Quinn, P. K.; Sierau, B.

    2007-01-01

    We have determined the solar spectral absorption optical depth of atmospheric aerosols for specific case studies during several field programs (three cases have been reported previously; two are new results). We combined airborne measurements of the solar net radiant flux density and the aerosol optical depth with a detailed radiative transfer model for all but one of the cases. The field programs (SAFARI 2000, ACE Asia, PRIDE, TARFOX, INTEX-A) contained aerosols representing the major absorbing aerosol types: pollution, biomass burning, desert dust and mixtures. In all cases the spectral absorption optical depth decreases with wavelength and can be approximated with a power-law wavelength dependence (Absorption Angstrom Exponent or AAE). We compare our results with other recent spectral absorption measurements and attempt to briefly summarize the state of knowledge of aerosol absorption spectra in the atmosphere. We discuss the limitations in using the AAE for calculating the solar absorption. We also discuss the resulting spectral single scattering albedo for these cases.

  2. A satellite view of aerosols in the climate system

    NASA Technical Reports Server (NTRS)

    Kaufman, Yoram J.; Tanre, Didier; Boucher, Olivier

    2002-01-01

    Anthropogenic aerosols are intricately linked to the climate system and to the hydrologic cycle. The net effect of aerosols is to cool the climate system by reflecting sunlight. Depending on their composition, aerosols can also absorb sunlight in the atmosphere, further cooling the surface but warming the atmosphere in the process. These effects of aerosols on the temperature profile, along with the role of aerosols as cloud condensation nuclei, impact the hydrologic cycle, through changes in cloud cover, cloud properties and precipitation. Unravelling these feedbacks is particularly difficult because aerosols take a multitude of shapes and forms, ranging from desert dust to urban pollution, and because aerosol concentrations vary strongly over time and space. To accurately study aerosol distribution and composition therefore requires continuous observations from satellites, networks of ground-based instruments and dedicated field experiments. Increases in aerosol concentration and changes in their composition, driven by industrialization and an expanding population, may adversely affect the Earth's climate and water supply.

  3. Long-term profiling of mineral dust and pollution aerosol with multiwavelength polarization Raman lidar at the Central Asian site of Dushanbe, Tajikistan: case studies

    NASA Astrophysics Data System (ADS)

    Hofer, Julian; Althausen, Dietrich; Abdullaev, Sabur F.; Makhmudov, Abduvosit N.; Nazarov, Bakhron I.; Schettler, Georg; Engelmann, Ronny; Baars, Holger; Wadinga Fomba, K.; Müller, Konrad; Heinold, Bernd; Kandler, Konrad; Ansmann, Albert

    2017-12-01

    For the first time, continuous vertically resolved aerosol measurements were performed by lidar in Tajikistan, Central Asia. Observations with the multiwavelength polarization Raman lidar PollyXT were conducted during CADEX (Central Asian Dust EXperiment) in Dushanbe, Tajikistan, from March 2015 to August 2016. Co-located with the lidar, a sun photometer was also operated. The goal of CADEX is to provide an unprecedented data set on vertically resolved aerosol optical properties in Central Asia, an area highly affected by climate change but largely missing vertically resolved aerosol measurements. During the 18-month measurement campaign, mineral dust was detected frequently from ground to the cirrus level height. In this study, an overview of the measurement period is given and four typical but different example measurement cases are discussed in detail. Three of them are dust cases and one is a contrasting pollution aerosol case. Vertical profiles of the measured optical properties and the calculated dust and non-dust mass concentrations are presented. Dust source regions were identified by means of backward trajectory analyses. A lofted layer of Middle Eastern dust with an aerosol optical thickness (AOT) of 0.4 and an extinction-related Ångström exponent of 0.41 was measured. In comparison, two near-ground dust cases have Central Asian sources. One is an extreme dust event with an AOT of 1.5 and Ångström exponent of 0.12 and the other one is a most extreme dust event with an AOT of above 4 (measured by sun photometer) and an Ångström exponent of -0.08. The observed lidar ratios (and particle linear depolarization ratios) in the presented dust cases range from 40.3 to 46.9 sr (and 0.18-0.29) at 355 nm and from 35.7 to 42.9 sr (0.31-0.35) at 532 nm wavelength. The particle linear depolarization ratios indicate almost unpolluted dust in the case of a lofted dust layer and pure dust in the near-ground dust cases. The lidar ratio values are lower than typical

  4. The Relationship between Aerosol Composition and Concentration and Visual Range on Barbados, West Indies: The Impact of African Dust

    NASA Astrophysics Data System (ADS)

    Huang, J.; Prospero, J.; Zhang, C.; Arimoto, R.

    2006-12-01

    Visual Range (VR) measured at Grantley Adams Airport on Barbados shows a very strong annual cycle with the minimum VR values occurring in June or July. This cycle closely matches the annual cycle of African dust concentrations measured in the trade winds at Barbados (13°15'N, 59°30'W) where observations first began in 1965. In winter, monthly mean VR was typically around 30 km or greater while in summer it frequently dipped below 20 km. This same clear signal is observed in the VR records from near-by islands where the same seasonal cycle of dust would be expected: St. Lucia, Martinique and Trinidad and Tobago. We examined the relationship between VR on Barbados and the concentrations of the three major aerosol constituents that we would expect to have the strongest influence on VR: mineral dust, sea salt, and non-sea- salt sulfate (nss-SO4^{=}). We used VR data for the period from 1973, when measurements first began, up to 2006. We found a large discrepancy between the observed VR at the airport and the VR derived from the Koschmieder equation using literature values for the optical properties of the aerosol components; this simple approach would require a much smaller constant than the commonly-used value, 3.912. We further explored the effects of particle size distribution and relative humidity. During boreal summer when VR is lowest, dust is the dominant supramicron aerosol component and it clearly is the major factor in controlling VR. Nonetheless the submicron fraction also has a comparable impact due to its significantly higher light scattering efficiency. During winter, when there is little or no dust, sea salt aerosol and sulfate are dominant. In this report we focus on the various factors that affect visibility on Barbados especially the role of aerosols dominated by supramicrometer particles. We also consider the effects of other factors such as wind speed and precipitation. Finally, we note that the close relationship between summertime VR and dust

  5. Remote sensing of desert dust aerosols over the Sahel : potential use for health impact studies

    NASA Astrophysics Data System (ADS)

    Deroubaix, A. D.; Martiny, N. M.; Chiapello, I. C.; Marticorena, B. M.

    2012-04-01

    Since the end of the 70's, remote sensing monitors the desert dust aerosols due to their absorption and scattering properties and allows to make long time series which are necessary for air quality or health impact studies. In the Sahel, a huge health problem is the Meningitis Meningococcal (MM) epidemics that occur during the dry season : the dust has been suspected to be crucial to understand their onsets and dynamics. The Aerosol absorption Index (AI) is a semi-quantitative index derived from TOMS and OMI observations in the UV available at a spatial resolution of 1° (1979-2005) and 0.25° (2005-today) respectively. The comparison of the OMI-AI and AERONET Aerosol Optical thickness (AOT) shows a good agreement at a daily time-step (correlation ~0.7). The comparison of the OMI-AI with the Particle Matter (PM) measurement of the Sahelian Dust Transect is lower (~0.4) at a daily time-step but it increases at a weekly time-step (~0.6). The OMI-AI reproduces the dust seasonal cycle over the Sahel and we conclude that the OMI-AI product at a 0.25° spatial resolution is suitable for health impact studies, especially at a weekly epidemiological time-step. Despite the AI is sensitive to the aerosol altitude, it provides a daily spatial information on dust. A preliminary investigation analysis of the link between weekly OMI AI and weekly WHO epidemiological data sets is presented in Mali and Niger, showing a good agreement between the AI and the onset of the MM epidemics with a constant lag (between 1 and 2 week). The next of this study is to analyse a deeper AI time series constituted by TOMS and OMI data sets. Based on the weekly ratios PM/AI at 2 stations of the Sahelian Dust Transect, a spatialized proxy for PM from the AI has been developed. The AI as a proxy for PM and other climate variables such as Temperature (T°), Relative Humidity (RH%) and the wind (intensity and direction) could then be used to analyze the link between those variables and the MM epidemics

  6. Optical properties and aging of light-absorbing secondary organic aerosol

    DOE PAGES

    Liu, Jiumeng; Lin, Peng; Laskin, Alexander; ...

    2016-10-14

    The light-absorbing organic aerosol (OA) commonly referred to as “brown carbon” (BrC) has attracted considerable attention in recent years because of its potential to affect atmospheric radiation balance, especially in the ultraviolet region and thus impact photochemical processes. A growing amount of data has indicated that BrC is prevalent in the atmosphere, which has motivated numerous laboratory and field studies; however, our understanding of the relationship between the chemical composition and optical properties of BrC remains limited. We conducted chamber experiments to investigate the effect of various volatile organic carbon (VOC) precursors, NO x concentrations, photolysis time, and relative humidity (RH) on the lightmore » absorption of selected secondary organic aerosols (SOA). Light absorption of chamber-generated SOA samples, especially aromatic SOA, was found to increase with NO x concentration, at moderate RH, and for the shortest photolysis aging times. The highest mass absorption coefficient (MAC) value is observed from toluene SOA products formed under high-NO x conditions at moderate RH, in which nitro-aromatics were previously identified as the major light-absorbing compounds. BrC light absorption is observed to decrease with photolysis time, correlated with a decline of the organic nitrate fraction of SOA. SOA formed from mixtures of aromatics and isoprene absorb less visible (Vis) and ultraviolet (UV) light than SOA formed from aromatic precursors alone on a mass basis. However, the mixed SOA absorption was underestimated when optical properties were predicted using a two-product SOA formation model, as done in many current climate models. Further investigation, including analysis on detailed mechanisms, are required to explain the discrepancy.« less

  7. Optical Properties and Aging of Light Absorbing Secondary Organic Aerosol

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Liu, Jiumeng; Lin, Peng; Laskin, Alexander

    2016-10-14

    The light-absorbing organic aerosol (OA), commonly referred to as “brown carbon (BrC)”, has attracted considerable attention in recent years because of its potential to affect atmospheric radiation balance, especially in the ultraviolet region and thus impact photochemical processes. A growing amount of data has indicated that BrC is prevalent in the atmosphere, which has motivated numerous laboratory and field studies; however, our understanding of the relationship between the chemical composition and optical properties of BrC remains limited. We conducted chamber experiments to investigate the effect of various VOC precursors, NOx concentrations, photolysis time and relative humidity (RH) on the lightmore » absorption of selected secondary organic aerosols (SOA). Light absorption of chamber generated SOA samples, especially aromatic SOA, was found to increase with NOx concentration, at moderate RH, and for the shortest photolysis aging times. The highest mass absorption coefficients (MAC) value is observed from toluene SOA products formed under high NOx conditions at moderate RH, in which nitro-aromatics were previously identified as the major light absorbing compounds. BrC light absorption is observed to decrease with photolysis time, correlated with a decline of the organonitrate fraction of SOA. SOA formed from mixtures of aromatics and isoprene absorb less visible and UV light than SOA formed from aromatic precursors alone on a mass basis. However, the mixed-SOA absorption was underestimated when optical properties were predicted using a two-product SOA formation model, as done in many current climate models. Further investigation, including analysis on detailed mechanisms, are required to explain the discrepancy.« less

  8. Atmospheric correction of SeaWiFS ocean color imagery in the presence of absorbing aerosols off the Indian coast using a neuro-variational method

    NASA Astrophysics Data System (ADS)

    Brajard, J.; Moulin, C.; Thiria, S.

    2008-10-01

    This paper presents a comparison of the atmospheric correction accuracy between the standard sea-viewing wide field-of-view sensor (SeaWiFS) algorithm and the NeuroVaria algorithm for the ocean off the Indian coast in March 1999. NeuroVaria is a general method developed to retrieve aerosol optical properties and water-leaving reflectances for all types of aerosols, including absorbing ones. It has been applied to SeaWiFS images of March 1999, during an episode of transport of absorbing aerosols coming from pollutant sources in India. Water-leaving reflectances and aerosol optical thickness estimated by the two methods were extracted along a transect across the aerosol plume for three days. The comparison showed that NeuroVaria allows the retrieval of oceanic properties in the presence of absorbing aerosols with a better spatial and temporal stability than the standard SeaWiFS algorithm. NeuroVaria was then applied to the available SeaWiFS images over a two-week period. NeuroVaria algorithm retrieves ocean products for a larger number of pixels than the standard one and eliminates most of the discontinuities and artifacts associated with the standard algorithm in presence of absorbing aerosols.

  9. Light absorption by secondary organic aerosol from α-pinene: Effects of oxidants, seed aerosol acidity, and relative humidity

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Song, Chen; Gyawali, Madhu; Zaveri, Rahul A.

    2013-10-25

    It is well known that light absorption from dust and black carbon aerosols has a warming effect on climate while light scattering from sulfate, nitrate, and sea salt aerosols has a cooling effect. However, there are large uncertainties associated with light absorption and scattering by different types of organic aerosols, especially in the near-UV and UV spectral regions. In this paper, we present the results from a systematic laboratory study focused on measuring light absorption by secondary organic aerosols (SOAs) generated from dark α-pinene + O 3 and α-pinene + NO x + O 3 systems in the presence ofmore » neutral and acidic sulfate seed aerosols. Light absorption was monitored using photoacoustic spectrometers at four different wavelengths: 355, 405, 532, and 870 nm. Significant light absorption at 355 and 405 nm was observed for the SOA formed from α-pinene + O 3 + NO 3 system only in the presence of highly acidic sulfate seed aerosols under dry conditions. In contrast, no absorption was observed when the relative humidity was elevated to greater than 27% or in the presence of neutral sulfate seed aerosols. Organic nitrates in the SOA formed in the presence of neutral sulfate seed aerosols were found to be nonabsorbing, while the light-absorbing compounds are speculated to be aldol condensation oligomers with nitroxy organosulfate groups that are formed in highly acidic sulfate aerosols. Finally and overall, these results suggest that dark α-pinene + O 3 and α-pinene + NO x + O 3 systems do not form light-absorbing SOA under typical atmospheric conditions.« less

  10. Retrieval of Aerosol Absorption Properties from Satellite Observations

    NASA Technical Reports Server (NTRS)

    Torres, Omar; Bhartia, Pawan K.; Jethva, H.; Ahn, Chang-Woo

    2012-01-01

    The Angstrom Absorption Exponent (AAE) is a parameter commonly used to characterize the wavelength-dependence of aerosol absorption optical depth (AAOD). It is closely related to aerosol composition. Black carbon (BC) containing aerosols yield AAE values near unity whereas Organic carbon (OC) aerosol particles are associated with values larger than 2. Even larger AAE values have been reported for desert dust aerosol particles. Knowledge of spectral AAOD is necessary for the calculation of direct radiative forcing effect of aerosols and for inferring aerosol composition. We have developed a satellitebased method of determining the spectral AAOD of absorbing aerosols. The technique uses multi-spectral measurements of upwelling radiation from scenes where absorbing aerosols lie above clouds as indicated by the UV Aerosol Index. For those conditions, the satellite measurement can be explained, using an approximations of Beer's Law (BL), as the upwelling reflectance at the cloud top attenuated by the absorption effects of the overlying aerosol layer. The upwelling reflectance at the cloud-top in an aerosol-free atmospheric column is mainly a function of cloud optical depth (COD). In the proposed method of AAE derivation, the first step is determining COD which is retrieved using a previously developed color-ratio based approach. In the second step, corrections for molecular scattering effects are applied to both the observed ad the calculated cloud reflectance terms, and the spectral AAOD is then derived by an inversion of the BL approximation. The proposed technique will be discussed in detail and application results making use of OMI multi-spectral measurements in the UV-Vis. will be presented.

  11. Dust, Pollution, and Biomass Burning Aerosols in Asian Pacific: A Column Satellite-Surface Perspective

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee

    2004-01-01

    Airborne dusts from northern China contribute a significant part of the air quality problem and, to some extent, regional climatic impact in Asia during spring-time. However, with the economical growth in China, increases in the emission of air pollutants generated from industrial and vehicular sources will not only impact the radiation balance, but adverse health effects to humans all year round. In addition, both of these dust and air pollution clouds can transport swiftly across the Pacific reaching North America within a few days, possessing an even larger scale effect. The Asian dust and air pollution aerosols can be detected by its colored appearance on current Earth observing satellites (e.g., MODIS, SeaWiFS, TOMS, etc.) and its evolution monitored by satellites and surface network. Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially those in Africa, South America, and Southeast Asia. However, the unique climatology of Southeast Asia is very different than that of Africa and South America, such that large-scale biomass burning causes smoke to interact extensively with clouds during the peak-burning season of March to April. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass burning processes. These gases influence the Earth-atmosphere system, impacting both global climate and tropospheric chemistry. Some aerosols can serve as cloud condensation nuclei, which play an important role in determining cloud lifetime and precipitation, hence, altering the earth's radiation and water budget. Biomass burning also affects the biogeochemical cycling of nitrogen and carbon compounds from the soil to the atmosphere; the hydrological cycle (i.e., run off and evaporation); land surface reflectivity and emissivity; as well as ecosystem biodiversity and stability. Two new initiatives, EAST-AIRE (East

  12. Why Is Improvement of Earth System Models so Elusive? Challenges and Strategies from Dust Aerosol Modeling

    NASA Technical Reports Server (NTRS)

    Miller, Ronald L.; Garcia-Pando, Carlos Perez; Perlwitz, Jan; Ginoux, Paul

    2015-01-01

    Past decades have seen an accelerating increase in computing efficiency, while climate models are representing a rapidly widening set of physical processes. Yet simulations of some fundamental aspects of climate like precipitation or aerosol forcing remain highly uncertain and resistant to progress. Dust aerosol modeling of soil particles lofted by wind erosion has seen a similar conflict between increasing model sophistication and remaining uncertainty. Dust aerosols perturb the energy and water cycles by scattering radiation and acting as ice nuclei, while mediating atmospheric chemistry and marine photosynthesis (and thus the carbon cycle). These effects take place across scales from the dimensions of an ice crystal to the planetary-scale circulation that disperses dust far downwind of its parent soil. Representing this range leads to several modeling challenges. Should we limit complexity in our model, which consumes computer resources and inhibits interpretation? How do we decide if a process involving dust is worthy of inclusion within our model? Can we identify a minimal representation of a complex process that is efficient yet retains the physics relevant to climate? Answering these questions about the appropriate degree of representation is guided by model evaluation, which presents several more challenges. How do we proceed if the available observations do not directly constrain our process of interest? (This could result from competing processes that influence the observed variable and obscure the signature of our process of interest.) Examples will be presented from dust modeling, with lessons that might be more broadly applicable. The end result will either be clinical depression or there assuring promise of continued gainful employment as the community confronts these challenges.

  13. Observational Evidence of Impacts of Aerosols on Seasonal-to-Interannual Variability of the Asian Monsoon

    NASA Technical Reports Server (NTRS)

    Lau, K.-M.; Kim, K.-M.; Hsu, N. C.

    2006-01-01

    Observational evidences are presented showing that the Indian subcontinent and surrounding regions are subject to heavy loading of absorbing aerosols (dust and black carbon), with strong seasonality closely linked to the monsoon annual rainfall cycle. Increased loading of absorbing aerosols over the Indo-Gangetic Plain in April-May is associated with a) increased heating of the upper troposphere over the Tibetan Plateau, b) an advance of the monsoon rainy season, and c) subsequent enhancement of monsoon rainfall over the South Asia subcontinent, and reduction over East Asia. Also presented are radiative transfer calculations showing how differential solar absorption by aerosols over bright surface (desert or snow cover land) compared to dark surface (vegetated land and ocean), may be instrumental in triggering an aerosol-monsoon large-scale circulation and water cycle feedback, consistent with the elevated heat pump hypothesis (Lau et al. 2006).

  14. Dust-wind interactions can intensify aerosol pollution over eastern China

    DOE PAGES

    Yang, Yang; Russell, Lynn M.; Lou, Sijia; ...

    2017-05-11

    Eastern China has experienced severe and persistent winter haze episodes in recent years due to intensification of aerosol pollution, which has adverse impacts on hundreds of millions of people across China1–4. In addition to anthropogenic emissions, the winter aerosol pollution over eastern China is associated with abnormal meteorological conditions, including weaker wind speeds5–9. Using a global climate model and a chemical transport model, we show that variations in dust emissions decrease the wintertime land-sea surface air temperature difference between eastern China and the South China Sea and weaken winds below the lowest 10th percentile of wind speed by 0.06 mmore » s-1. Here, the weakened winds enhance stagnation and account for 13% of the increases in PM2.5 aerosol concentrations over eastern China. Although recent increases in anthropogenic emissions are the main factor causing haze over eastern China, we conclude that natural emissions also exert a significant influence on the increases in wintertime PM2.5 concentrations, with important implications that should be considered in air quality studies.« less

  15. Dust-wind interactions can intensify aerosol pollution over eastern China

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yang, Yang; Russell, Lynn M.; Lou, Sijia

    Eastern China has experienced severe and persistent winter haze episodes in recent years due to intensification of aerosol pollution, which has adverse impacts on hundreds of millions of people across China1–4. In addition to anthropogenic emissions, the winter aerosol pollution over eastern China is associated with abnormal meteorological conditions, including weaker wind speeds5–9. Using a global climate model and a chemical transport model, we show that variations in dust emissions decrease the wintertime land-sea surface air temperature difference between eastern China and the South China Sea and weaken winds below the lowest 10th percentile of wind speed by 0.06 mmore » s-1. Here, the weakened winds enhance stagnation and account for 13% of the increases in PM2.5 aerosol concentrations over eastern China. Although recent increases in anthropogenic emissions are the main factor causing haze over eastern China, we conclude that natural emissions also exert a significant influence on the increases in wintertime PM2.5 concentrations, with important implications that should be considered in air quality studies.« less

  16. Long-term systematic profiling of dust aerosol optical properties using the EOLE NTUA lidar system over Athens, Greece (2000-2016)

    NASA Astrophysics Data System (ADS)

    Soupiona, O.; Papayannis, A.; Kokkalis, P.; Mylonaki, M.; Tsaknakis, G.; Argyrouli, A.; Vratolis, S.

    2018-06-01

    We present a comprehensive analysis of the seasonal variability of the vertical profiles of the optical and geometrical properties of Saharan dust aerosols, observed in the height region between 1000 and 6000 m, over the city of Athens, Greece, from February 2000 to December 2016. These observations were performed by a multi-wavelength (355-387-532-1064 nm) Raman lidar system under cloud-free conditions. The statistical analysis (using aerosol monthly mean values) is based on nighttime vertical Raman measurements of range-resolved aerosol optical properties (backscatter and extinction coefficients, lidar ratio, Ångström exponent) at 355 nm (57 dust events during more than 80 measurement hours). We found that the number of dust events was highest in spring, summer, and early autumn periods and that during spring the dust layers were moved at higher altitudes (∼4500 m) than in other seasons. The number of the forecasted dusty days (on monthly basis) by the BSC-DREAM8b model compared to those of the performed lidar measurements were found to have a quite strong correlation (R2 = 0.81), with a maximum occurrence predicted for the spring season. In the worst case scenario, at least 50% of the model-forecasted dust events can be observed by lidar under cloudless skies over Athens. For the sampled dust plumes we found mean lidar ratios of 52 ± 13 sr at 355 nm in the height range 2000-4000 m a.s.l. Moreover, the dust layers had a mean thickness of 2497 ± 1026 m and a center of mass of 2699 ± 1017 m. An analysis performed regarding the air mass back-trajectories arriving over Athens revealed two main clusters: one pathway from south-west to north-east, with dust emission areas in Tunisia, Algeria and Libya and a second one from south, across the Mediterranean Sea with emission areas over Libya and the remaining part of Algeria and Tunisia. This clustering enabled us to differentiate between the aerosol optical properties between the two clusters, based on their

  17. Impact of long-range transport pollution on aerosol properties over West Africa: observations during the DACCIWA airborne campaign

    NASA Astrophysics Data System (ADS)

    Denjean, Cyrielle; Bourrianne, Thierry; Burnet, Frederic; Deroubaix, Adrien; Brito, Joel; Dupuy, Régis; Colomb, Aurélie; Schwarzenboeck, Alfons; Sellegri, Karine; Chazette, Patrick; Duplissy, Jonathan; Flamant, Cyrille

    2017-04-01

    Southern West Africa (SWA) is a region highly vulnerable to climate change. Emissions of anthropogenic pollution have increased substantially over the past decades in the region and are projected to keep increasing. The region is also strongly impacted by important natural pollution from distant locations. Biomass burning mainly from vegetation fires in Central Africa and mineral dust from the Saharan and Sahel-Sudan regions are advected by winds to the SWA region especially in summer. Both biomass burning and mineral dust aerosols scatter and absorb solar radiation and are able to significantly modify the regional radiative budget. Presently, the potential radiative impact of dust and biomass burning particles on SWA is unclear due to inadequate data information on the aerosols properties and vertical distribution. In the framework of the Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa (DACCIWA) project, an unprecedented field campaign took place in summer 2016 in West Africa. The ATR-42 research aircraft operated by SAFIRE performed twenty flights to sample the local air pollution from maritime traffic and coastal megacities, as well as regional pollution from biomass burning and desert dust. The aircraft was equipped with state of the art in situ instrumentation to measure the aerosol optical properties (CAPS, nephelometer, PSAP), the aerosol size distribution (SMPS, GRIMM, USHAS, PCASP, FSSP) and the aerosol chemical composition (SP2, AMS). A mini backscattered lidar system provided additional measurements of the aerosol vertical structure and the aerosol optical properties such as the particulate depolarization ratio. The CHIMERE chemistry and transport model has been used to characterize the source area and the long-range transport of dust and biomass burning plumes. Here, we investigate the aerosol microphysical, chemical and optical properties of biomass burning and dust aerosols transported in SWA. In particular the following questions will be

  18. Size-segregated sugar composition of transported dust aerosols from Middle-East over Delhi during March 2012

    NASA Astrophysics Data System (ADS)

    Kumar, S.; Aggarwal, S. G.; Fu, P. Q.; Kang, M.; Sarangi, B.; Sinha, D.; Kotnala, R. K.

    2017-06-01

    During March 20-22, 2012 Delhi experienced a massive dust-storm which originated in Middle-East. Size segregated sampling of these dust aerosols was performed using a nine staged Andersen sampler (5 sets of samples were collected including before dust-storm (BDS)), dust-storm day 1 to 3 (DS1 to DS3) and after dust storm (ADS). Sugars (mono and disaccharides, sugar-alcohols and anhydro-sugars) were determined using GC-MS technique. It was observed that on the onset of dust-storm, total suspended particulate matter (TSPM, sum of all stages) concentration in DS1 sample increased by > 2.5 folds compared to that of BDS samples. Interestingly, fine particulate matter (sum of stages with cutoff size < 2.1 μm) loading in DS1 also increased by > 2.5 folds as compared to that of BDS samples. Sugars analyzed in DS1 coarse mode (sum of stages with cutoff size > 2.1 μm) samples showed a considerable increase ( 1.7-2.8 folds) compared to that of other samples. It was further observed that mono-saccharides, disaccharides and sugar-alcohols concentrations were enhanced in giant (> 9.0 μm) particles in DS1 samples as compared to other samples. On the other hand, anhydro-sugars comprised 13-27% of sugars in coarse mode particles and were mostly found in fine mode constituting 66-85% of sugars in all the sample types. Trehalose showed an enhanced ( 2-4 folds) concentration in DS1 aerosol samples in both coarse (62.80 ng/m3) and fine (8.57 ng/m3) mode. This increase in Trehalose content in both coarse and fine mode suggests their origin to the transported desert dust and supports their candidature as an organic tracer for desert dust entrainments. Further, levoglucosan to mannosan (L/M) ratios which have been used to predict the type of biomass burning influences on aerosols are found to be size dependent in these samples. These ratios are higher for fine mode particles, hence should be used with caution while interpreting the sources using this tool.

  19. Dust and Smoke

    Atmospheric Science Data Center

    2014-05-15

    ...     View Larger Image Desert dust particles tend to be larger in size than aerosols that originate ... for these two events. These MISR results distinguish desert dust, the most common non-spherical aerosol type, from pollution and ...

  20. Characterizing dust aerosols in the atmospheric boundary layer over the deserts in Northwest China: monitoring network and field observation

    NASA Astrophysics Data System (ADS)

    He, Q.; Matimin, A.; Yang, X.

    2016-12-01

    TheTaklimakan, Gurbantunggut and BadainJaran Deserts with the total area of 43.8×104 km2 in Northwest China are the major dust emission sources in Central Asia. Understanding Central Asian dust emissions and the interaction with the atmospheric boundary layer has an important implication for regional and global climate and environment changes. In order to explore these scientific issues, a monitoring network of 63 sites was established over the vast deserts (Taklimakan Desert, Gurbantunggut Desert and Badain Jaran Desert) in Northwest China for the comprehensive measurements of dust aerosol emission, transport and deposition as well as the atmospheric boundary layer including the meteorological parameters of boundary layer, surface radiation, surface heat fluxes, soil parameters, dust aerosol properties, water vapor profiles, and dust emission. Based on the monitoring network, the field experiments have been conducted to characterize dust aerosols and the atmospheric boundary layer over the deserts. The experiment observation indicated that depth of the convective boundary layer can reach 5000m on summer afternoons. In desert regions, the diurnal mean net radiation was effected significantly by dust weather, and sensible heat was much greater than latent heat accounting about 40-50% in the heat balance of desert. The surface soil and dust size distributions of Northwest China Deserts were obtained through widely collecting samples, results showed that the dominant dust particle size was PM100within 80m height, on average accounting for 60-80% of the samples, with 0.9-2.5% for PM0-2.5, 3.5-7.0% for PM0-10 and 5.0-14.0% for PM0-20. The time dust emission of Taklimakan Desert, Gurbantunggut Desert and Badain Jaran Desert accounted for 0.48%, 7.3%×10-5and 1.9% of the total time within a year, and the threshold friction velocity for dust emission were 0.22-1.06m/s, 0.29-1.5m/s and 0.21-0.59m/s, respectively.

  1. Large Contribution of Coarse Mode to Aerosol Microphysical and Optical Properties: Evidence from Ground-Based Observations of a Transpacific Dust Outbreak at a High-Elevation North American Site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kassianov, E.; Pekour, M.; Flynn, C.

    Our work is motivated by previous studies of the long-range trans-Atlantic transport of Saharan dust and the observed quasi-static nature of coarse mode aerosol with a volume median diameter (VMD) of approximately 3.5 µm. We examine coarse mode contributions from the trans-Pacific transport of Asian dust to North American aerosol microphysical and optical properties using a dataset collected at the high-elevation, mountain-top Storm Peak Laboratory (SPL, 3.22 km above sea level [ASL]) and the nearby Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF, 2.76 km ASL). Data collected during the SPL Cloud Property Validation Experiment (STORMVEX, March 2011) are complemented bymore » quasi-global high-resolution model simulations coupled with aerosol chemistry. We identify dust event associated mostly with Asian plume (about 70% of dust mass) where the coarse mode with moderate (~4 µm) VMD is distinct and contributes substantially to aerosol microphysical (up to 70% for total volume) and optical (up to 45% for total scattering and aerosol optical depth) properties. Our results, when compared with previous Saharan dust studies, suggest a fairly invariant behavior of coarse mode dust aerosols. If confirmed in additional studies, this invariant behavior may simplify considerably model parameterizations for complex and size-dependent processes associated with dust transport and removal.« less

  2. Laboratory study of the effect of oxalic acid on the cloud condensation nuclei activity of mineral dust aerosol

    NASA Astrophysics Data System (ADS)

    Gierlus, Kelly M.; Laskina, Olga; Abernathy, Tricia L.; Grassian, Vicki H.

    2012-01-01

    Dicarboxylic acids, which make up a significant portion of the atmospheric organic aerosol, are emitted directly through biomass burning as well as produced through the oxidation of volatile organic compounds. Oxalic acid, the most abundant of the dicarboxylic acids, has been shown by recent field studies to be present in mineral dust aerosol particles. The presence of these internally mixed organic compounds can alter the water absorption and cloud condensation nuclei (CCN) abilities of mineral particles in the Earth's atmosphere. The University of Iowa's Multi-Analysis Aerosol Reactor System ( MAARS) was used to measure the CCN activity of internally mixed particles that were generated from a mixture of either calcite or polystyrene latex spheres (PSLs) in an aqueous solution of oxalic acid. Although PSL is not a mineral dust component, it is used here as a non-reactive, insoluble particle. CCN measurements indicate that the internally mixed oxalate/calcite particles showed nearly identical CCN activity compared to the original calcite particles whereas oxalic acid/PSL internally mixed particles showed much greater CCN activity compared to PSL particles alone. This difference is due to the reaction of calcite with oxalic acid, which produces a relatively insoluble calcium oxalate coating on the particle surface and not a soluble coating as it does on the PSL particle. Our results suggest that atmospheric processing of mineral dust aerosol through heterogeneous processes will likely depend on the mineralogy and the specific chemistry involved. Increase in the CCN activity by incorporation of oxalic acid are only expected for unreactive insoluble dust particles that form a soluble coating.

  3. Spectral Aerosol Extinction (SpEx): A New Instrument for In situ Ambient Aerosol Extinction Measurements Across the UV/Visible Wavelength Range

    NASA Technical Reports Server (NTRS)

    Jordan, C. E.; Anderson, B. E.; Beyersdorf, A. J.; Corr, C. A.; Dibb, J. E.; Greenslade, M. E.; Martin, R. F.; Moore, R. H.; Scheuer, E.; Shook, M. A.; hide

    2015-01-01

    We introduce a new instrument for the measurement of in situ ambient aerosol extinction over the 300-700 nm wavelength range, the Spectral Aerosol Extinction (SpEx) instrument. This measurement capability is envisioned to complement existing in situ instrumentation, allowing for simultaneous measurement of the evolution of aerosol optical, chemical, and physical characteristics in the ambient environment. In this work, a detailed description of the instrument is provided along with characterization tests performed in the laboratory. Measured spectra of NO2 and polystyrene latex spheres agreed well with theoretical calculations. Good agreement was also found with simultaneous aerosol extinction measurements at 450, 530, and 630 nm using CAPS PMex instruments in a series of 22 tests including non-absorbing compounds, dusts, soot, and black and brown carbon analogs. SpEx can more accurately distinguish the presence of brown carbon from other absorbing aerosol due to its 300 nm lower wavelength limit compared to measurements limited to visible wavelengths. In addition, the spectra obtained by SpEx carry more information than can be conveyed by a simple power law fit that is typically defined by the use of Angstrom Exponents. Future improvements aim at lowering detection limits and ruggedizing the instrument for mobile operation.

  4. Informing Aerosol Transport Models With Satellite Multi-Angle Aerosol Measurements

    NASA Technical Reports Server (NTRS)

    Limbacher, J.; Patadia, F.; Petrenko, M.; Martin, M. Val; Chin, M.; Gaitley, B.; Garay, M.; Kalashnikova, O.; Nelson, D.; Scollo, S.

    2011-01-01

    As the aerosol products from the NASA Earth Observing System's Multi-angle Imaging SpectroRadiometer (MISR) mature, we are placing greater focus on ways of using the aerosol amount and type data products, and aerosol plume heights, to constrain aerosol transport models. We have demonstrated the ability to map aerosol air-mass-types regionally, and have identified product upgrades required to apply them globally, including the need for a quality flag indicating the aerosol type information content, that varies depending upon retrieval conditions. We have shown that MISR aerosol type can distinguish smoke from dust, volcanic ash from sulfate and water particles, and can identify qualitative differences in mixtures of smoke, dust, and pollution aerosol components in urban settings. We demonstrated the use of stereo imaging to map smoke, dust, and volcanic effluent plume injection height, and the combination of MISR and MODIS aerosol optical depth maps to constrain wildfire smoke source strength. This talk will briefly highlight where we stand on these application, with emphasis on the steps we are taking toward applying the capabilities toward constraining aerosol transport models, planet-wide.

  5. Dust Aerosol, Clouds, and the Atmospheric Optical Depth Record over 5 Mars Years of the Mars Exploration Rover Mission

    NASA Technical Reports Server (NTRS)

    Lemmon, Mark T.; Wolff, Michael J.; Bell, James F., III; Smith, Michael D.; Cantor, Bruce A.; Smith, Peter H.

    2014-01-01

    Dust aerosol plays a fundamental role in the behavior and evolution of the Martian atmosphere. The first five Mars years of Mars Exploration Rover data provide an unprecedented record of the dust load at two sites. This record is useful for characterization of the atmosphere at the sites and as ground truth for orbital observations. Atmospheric extinction optical depths have been derived from solar images after calibration and correction for time-varying dust that has accumulated on the camera windows. The record includes local, regional, and globally extensive dust storms. Comparison with contemporaneous thermal infrared data suggests significant variation in the size of the dust aerosols, with a 1 micrometer effective radius during northern summer and a 2 micrometer effective radius at the onset of a dust lifting event. The solar longitude (L (sub s)) 20-136 degrees period is also characterized by the presence of cirriform clouds at the Opportunity site, especially near LS = 50 and 115 degrees. In addition to water ice clouds, a water ice haze may also be present, and carbon dioxide clouds may be present early in the season. Variations in dust opacity are important to the energy balance of each site, and work with seasonal variations in insolation to control dust devil frequency at the Spirit site.

  6. Contrasting aerosol optical and radiative properties between dust and urban haze episodes in megacities of Pakistan

    NASA Astrophysics Data System (ADS)

    Iftikhar, Muhammad; Alam, Khan; Sorooshian, Armin; Syed, Waqar Adil; Bibi, Samina; Bibi, Humera

    2018-01-01

    Satellite and ground based remote sensors provide vital information about aerosol optical and radiative properties. Analysis of aerosol optical and radiative properties during heavy aerosol loading events in Pakistan are limited and, therefore, require in-depth examination. This work examines aerosol properties and radiative forcing during Dust Episodes (DE) and Haze Episodes (HE) between 2010 and 2014 over mega cities of Pakistan (Karachi and Lahore). Episodes having the daily averaged values of Aerosol Optical Depth (AOD) exceeding 1 were selected. DE were associated with high AOD and low Ångström Exponent (AE) over Karachi and Lahore while high AOD and high AE values were associated with HE over Lahore. Aerosol volume size distributions (AVSD) exhibited a bimodal lognormal distribution with a noticeable coarse mode peak at a radius of 2.24 μm during DE, whereas a fine mode peak was prominent at a radius 0.25 μm during HE. The results reveal distinct differences between HE and DE for spectral profiles of several parameters including Single Scattering Albedo (SSA), ASYmmetry parameter (ASY), and the real and imaginary components of refractive index (RRI and IRI). The AOD-AE correlation revealed that dust was the dominant aerosol type during DE and that biomass burning and urban/industrial aerosol types were pronounced during HE. Aerosol radiative forcing (ARF) was estimated using the Santa Barbra DISORT Atmospheric Radiative Transfer (SBDART) model. Calculations revealed a negative ARF at the Top Of the Atmosphere (ARFTOA) and at the Bottom Of the Atmosphere (ARFBOA), with positive ARF within the Atmosphere (ARFATM) during both DE and HE over Karachi and Lahore. Furthermore, estimations of ARFATM by SBDART were shown to be in good agreement with values derived from AERONET data for DE and HE over Karachi and Lahore.

  7. Impact of dust and smoke mixing on column-integrated aerosol properties from observations during a severe wildfire episode over Valencia (Spain).

    PubMed

    Gómez-Amo, J L; Estellés, V; Marcos, C; Segura, S; Esteve, A R; Pedrós, R; Utrillas, M P; Martínez-Lozano, J A

    2017-12-01

    The most destructive wildfire experienced in Spain since 2004 occurred close to Valencia in summer 2012. A total of 48.500ha were affected by two wildfires, which were mostly active during 29-30 June. The fresh smoke plume was detected at the Burjassot measurement station simultaneously to a severe dust episode. We propose an empirical method to evaluate the dust and smoke mixing and its impact on the microphysical and optical properties. For this, we combine direct-sun measurements with a Cimel CE-318 sun-photometer with an inversion methodology, and the Mie theory to derive the column-integrated size distribution, single scattering albedo (SSA) and asymmetry parameter (g). The mixing of dust and smoke greatly increased the aerosol load and modified the background aerosol properties. Mineral dust increased the aerosol optical depth (AOD) up to 1, while the smoke plume caused an extreme AOD peak of 8. The size distribution of the mixture was bimodal, with a fine and coarse modes dominated by the smoke particles and mineral dust, respectively. The SSA and g for the dust-smoke mixture show a marked sensitivity on the smoke mixing-ratio, mainly at longer wavelengths. Mineral dust and smoke share a similar SSA at 440nm (~0.90), but with opposite spectral dependency. A small dust contribution to the total AOD substantially affects the SSA of the mixture, and also SSA at 1020nm increases from 0.87 to 0.95. This leads to a different spectral behaviour of SSA that changes from positive (smoke plume) to negative (dust), depending on the dust and smoke mixing-ratio. Copyright © 2017 Elsevier B.V. All rights reserved.

  8. Climate Effects and Efficacy of Dust and Soot in Snow

    NASA Astrophysics Data System (ADS)

    Zender, C. S.; Flanner, M. G.; Randerson, J. T.; Mahowald, N. M.; Rasch, P. J.; Yoshioka, M.; Painter, T.

    2006-12-01

    Dust and industrial and biomass burning emissions from low and mid-latitudes dominate the absorbing impurities trapped in snow at mid- and high-latitudes. We study the effects of dust and smoke on global and regional climate using a general circulation model driven by observed and predicted aerosol emissions determined from satellite and in situ observations. The model has sophisticated treatments of aerosol and snowpack radiative and thermodynamic processes that compare well with observations of snow albedo evolution and impurity concentration. This presentation focuses on the individual and combined contributions of present day dust and soot to snow-albedo forcing and on the global temperature and snowpack responses. Results are emphasized near India and East Asia, where the anthropogenic aerosol forcing of surface albedo and hydrology is greatest. We find that dust and black carbon (BC) aerosols have climate change efficacies (surface temperature change per unit forcing) about 3--4 times greater than CO2, making them the most efficacious forcing agents known. We estimate present day dust and soot snowpack-forcing of ~ 0.050 W m-2 warms global climate by ~ 0.16 °K. Anthropogenic soot from fossil fuel sources causes more than 50% of this warming, and biomass burning can account for up to 30% in strong tropical or boreal burn years. The greatest forcings occur in the Tarim/Mongol region (due to dust), northeastern China (due to soot), and the Tibetan Plateau (both). Dirty springtime snow in these regions can darken albedo by more than 0.1 and increase surface absorption by more than 20 W m-2. These results have implications for the strength of the Asian Monsoon, which is negatively correlated with antecedent snow cover in non-ENSO years. Dust and soot have such strong efficacies because they increase spring melt rates thus reduce summer snow cover. In some regions and seasons, dirty snow reduces snowpack depth and cover by 50%, triggering strong snow and sea

  9. The analysis of in situ and retrieved aerosol properties measured during three airborne field campaigns

    NASA Astrophysics Data System (ADS)

    Corr, Chelsea A.

    Aerosols can directly influence climate, visibility, and photochemistry by scattering and absorbing solar radiation. Aerosol chemical and physical properties determine how efficiently a particle scatters and/or absorbs incoming short-wave solar radiation. Because many types of aerosol can act as nuclei for cloud droplets (CCN) and a smaller population of airborne particles facilitate ice crystal formation (IN), aerosols can also alter cloud-radiation interactions which have subsequent impacts on climate. Thus aerosol properties determine the magnitude and sign of both the direct and indirect impacts of aerosols on radiation-dependent Earth System processes. This dissertation will fill some gaps in our understanding of the role of aerosol properties on aerosol absorption and cloud formation. Specifically, the impact of aerosol oxidation on aerosol spectral (350nm < lambda< 500nm) absorption was examined for two biomass burning plumes intercepted by the NASA DC-S aircraft during the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) mission in Spring and Summer 2008. Spectral aerosol single scattering albedo (SSA) retrieved using actinic flux measured aboard the NASA DC-8 was used to calculate the aerosol absorption Angstrom exponents (AAE) for a 6-day-old plume on April 17 th and a 3-hour old plume on June 29th. Higher AAE values for the April 17th plume (6.78+/-0.38) indicate absorption by aerosol was enhanced in the ultraviolet relative to the visible portion of the short-wave spectrum in the older plume compared to the fresher plume (AAE= 3.34 0.11). These differences were largely attributed to the greater oxidation of the organic aerosol in the April 17th plume which can arise either from the aging of primary organic aerosol or the formation of spectrally-absorbing secondary organic aerosol. The validity of the actinic flux retrievals used above were also evaluated in this work by the comparison of SSA retrieved using

  10. Observations of Dust Using the NASA Geoscience Laser Altimeter System (GLAS): New New Measurements of Aerosol Vertical Distribution From Space

    NASA Technical Reports Server (NTRS)

    Welton, Ellsworth; Spinhirne, James D.; Palm, Steven P.; Hlavka, Dennis; Hart, William

    2003-01-01

    On January 12, 2003 NASA launched the first satellite-based lidar, the Geoscience Laser -Altimeter System (GLAS), onboard the ICESat spacecraft. The GLAS atmospheric measurements introduce a fundamentally new and important tool for understanding the atmosphere and climate. In the past, aerosols have only been studied from space using images gathered by passive sensors. Analysis of this passive data has lead to an improved understanding of aerosol properties, spatial distribution, and their effect on the earth's climate. However, these images do not show the aerosol's vertical distribution. As a result, a key piece of information has been missing. The measurements now obtained by GLAS will provide information on the vertical distribution of aerosols and clouds, and improve our ability to study their transport processes and aerosol-cloud interactions. Here we show an overview of GLAS, provide an update of its current status, and present initial observations of dust profiles. In particular, a strategy of characterizing the height profile of dust plumes over source regions will be presented.

  11. Impact of the 4 April 2014 Saharan dust outbreak on the photovoltaic power generation in Germany

    NASA Astrophysics Data System (ADS)

    Rieger, Daniel; Steiner, Andrea; Bachmann, Vanessa; Gasch, Philipp; Förstner, Jochen; Deetz, Konrad; Vogel, Bernhard; Vogel, Heike

    2017-11-01

    The importance for reliable forecasts of incoming solar radiation is growing rapidly, especially for those countries with an increasing share in photovoltaic (PV) power production. The reliability of solar radiation forecasts depends mainly on the representation of clouds and aerosol particles absorbing and scattering radiation. Especially under extreme aerosol conditions, numerical weather prediction has a systematic bias in the solar radiation forecast. This is caused by the design of numerical weather prediction models, which typically account for the direct impact of aerosol particles on radiation using climatological mean values and the impact on cloud formation assuming spatially and temporally homogeneous aerosol concentrations. These model deficiencies in turn can lead to significant economic losses under extreme aerosol conditions. For Germany, Saharan dust outbreaks occurring 5 to 15 times per year for several days each are prominent examples for conditions, under which numerical weather prediction struggles to forecast solar radiation adequately. We investigate the impact of mineral dust on the PV-power generation during a Saharan dust outbreak over Germany on 4 April 2014 using ICON-ART, which is the current German numerical weather prediction model extended by modules accounting for trace substances and related feedback processes. We find an overall improvement of the PV-power forecast for 65 % of the pyranometer stations in Germany. Of the nine stations with very high differences between forecast and measurement, eight stations show an improvement. Furthermore, we quantify the direct radiative effects and indirect radiative effects of mineral dust. For our study, direct effects account for 64 %, indirect effects for 20 % and synergistic interaction effects for 16 % of the differences between the forecast including mineral dust radiative effects and the forecast neglecting mineral dust.

  12. Aeolian Dust and Forest Fire Smoke in Urban Air

    NASA Astrophysics Data System (ADS)

    Brimblecombe, P.

    2006-12-01

    Particles of aeolian dust and forest fire smoke are now regularly detected in urban air. Although dusts are common on the Asian Pacific Rim and forest fire smoke characteristic of South East Asia they also frequently detected elsewhere. In the past dust was treated as though it was fairly inert and reactions on the surface limited to the neutralizing ability of alkaline minerals. More recent work shows that that dust has a complex organic chemistry. Observations in China found fatty acids from urban areas (oleic acid and linoleic acid from cooking) on dust derived aerosols. The fatty acids and PAHs decreased sharply after dust storms, suggesting a role for dust in removal processes. When silica particles absorb unsaturated compounds they can react with ozone and release compounds such as formaldehyde. Particles from forest fires have a similarly complex chemistry and the acid-alkaline balance may vary depend on the balance of removal rates of alkaline materials (ammonia, potassium carbonate) and inorganic and organic acids. Airborne dust and forest fire soot can contain humic like substances (HULIS) either as primary material or as secondary oxidation products of the surface of soot. This paper will report on the role polluted air masses in the generation humic materials, particularly those that are surface active. These materials of high molecular weight oxygen rich organic compounds, which exhibit a range of properties of importance in aerosols: they can form complexes with metal ions and thus enhance their solubility, photosensitize the oxidation of organic compounds and lower the surface tension of aqueous aerosols. HULIS can be oxidized to form a range of simpler acids such as formic, acetic and oxalic acid. Dust and forest fire smoke particles have a different composition and size range to that of typical urban combustion particles, so it is likely that the health impacts will be different, yet current regulation often does not recognize any significant

  13. Atmospheric Teleconnection over Eurasia Induced by Aerosol Radiative Forcing during Boreal Spring

    NASA Technical Reports Server (NTRS)

    Kim, Maeng-Ki; Lau, William K. M.; Chin, Mian; Kim, Kyu-Myong; Sud, Y. C.; Walker, Greg K.

    2006-01-01

    The direct effects of aerosols on global and regional climate during boreal spring are investigated based on numerical simulations with the NASA Global Modeling and Assimilation Office finite-volume general circulation model (fvGCM) with Microphyics of Clouds with the Relaxed Arakawa Schubert Scheme (McRAS), using aerosol forcing functions derived from the Goddard Ozone Chemistry Aerosol Radiation and Transport model (GOCART). The authors find that anomalous atmospheric heat sources induced by absorbing aerosols (dust and black carbon) excite a planetary-scale teleconnection pattern in sea level pressure, temperature, and geopotential height spanning North Africa through Eurasia to the North Pacific. Surface cooling due to direct effects of aerosols is found in the vicinity and downstream of the aerosol source regions, that is, South Asia, East Asia, and northern and western Africa. Significant atmospheric heating is found in regions with large loading of dust (over northern Africa and the Middle East) and black carbon (over Southeast Asia). Paradoxically, the most pronounced feature in aerosol-induced surface temperature is an east west dipole anomaly with strong cooling over the Caspian Sea and warming over central and northeastern Asia, where aerosol concentrations are low. Analyses of circulation anomalies show that the dipole anomaly is a part of an atmospheric teleconnection pattern driven by atmospheric heating anomalies induced by absorbing aerosols in the source regions, but the influence was conveyed globally through barotropic energy dispersion and sustained by feedback processes associated with the regional circulations. The surface temperature signature associated with the aerosol-induced teleconnection bears striking resemblance to the spatial pattern of observed long-term trend in surface temperature over Eurasia. Additionally, the boreal spring wave train pattern is similar to that reported by Fukutomi et al. associated with the boreal summer

  14. Light-absorbing Aerosol Properties in the Kathmandu Valley during SusKat-ABC Field Campaign

    NASA Astrophysics Data System (ADS)

    Kim, S.; Yoon, S.; Kim, J.; Cho, C.; Jung, J.

    2013-12-01

    Light-absorbing aerosols, such as black carbon (BC), are major contributors to the atmospheric heating and the reduction of solar radiation reaching at the earth's surface. In this study, we investigate light-absorption and scattering properties of aerosols (i.e., BC mass concentration, aerosol solar-absorption/scattering efficiency) in the Kathmandu valley during Sustainable atmosphere for the Kathmandu valley (SusKat)-ABC campaign, from December 2012 to February 2013. Kathmandu City is among the most polluted cities in the world. However, there are only few past studies that provide basic understanding of air pollution in the Kathmandu Valley, which is not sufficient for designing effective mitigation measures (e.g., technological, financial, regulatory, legal and political measures, planning strategies). A distinct diurnal variation of BC mass concentration with two high peaks observed during wintertime dry monsoon period. BC mass concentration was found to be maximum around 09:00 and 20:00 local standard time (LST). Increased cars and cooking activities including substantial burning of wood and other biomass in the morning and in the evening contributed to high BC concentration. Low BC concentrations during the daytime can be explain by reduced vehicular movement and cooking activities. Also, the developmements of the boundary layer height and mountain-valley winds in the Kathmandu Valley paly a crucial role in the temproal variation of BC mass concentrations. Detailed radiative effects of light-absorbing aerosols will be presented.

  15. Dust transport over the eastern Mediterranean derived from Total Ozone Mapping Spectrometer, Aerosol Robotic Network, and surface measurements

    NASA Astrophysics Data System (ADS)

    Kalivitis, N.; Gerasopoulos, E.; Vrekoussis, M.; Kouvarakis, G.; Kubilay, N.; Hatzianastassiou, N.; Vardavas, I.; Mihalopoulos, N.

    2007-02-01

    Multiyear surface PM10 measurements performed on Crete Island, Greece, have been used in conjunction with satellite (Total Ozone Mapping Spectrometer (TOMS)) and ground-based remote sensing measurements (Aerosol Robotic Network (AERONET)) to enhance our understanding of the evolution of mineral dust events over the eastern Mediterranean. An analysis of southerly air masses at altitudes of 1000 and 3000 m over a 5 year period (2000-2005), showed that dust can potentially arrive over Crete, either simultaneously in the lower free troposphere and inside the boundary layer (vertical extended transport (VET)) or initially into the free troposphere with the heavier particles gradually being scavenged inside the boundary layer (free troposphere transport (FTT)). Both pathways present significant seasonal variations but on an annual basis contribute almost equally to the dust transport in the area. During VET the aerosol index (AI) derived from TOMS was significantly correlated with surface PM10, and in general AI was found to be adequate for the characterization of dust loadings over the eastern Mediterranean on a climatological basis. A significant covariance between PM10 and AOT was observed during VET as well, indicating that AOT levels from AERONET may be estimated by PM10 levels at the surface. Surface measurements are thus crucial for the validation of remote sensing measurements and hence are a powerful tool for the investigation of the impact of aerosols on climate.

  16. Remote sensing of mineral dust aerosol using AERI during the UAE2: A modeling and sensitivity study

    NASA Astrophysics Data System (ADS)

    Hansell, R. A.; Liou, K. N.; Ou, S. C.; Tsay, S. C.; Ji, Q.; Reid, J. S.

    2008-09-01

    Numerical simulations and sensitivity studies have been performed to assess the potential for using brightness temperature spectra from a ground-based Atmospheric Emitted Radiance Interferometer (AERI) during the United Arab Emirates Unified Aerosol Experiment (UAE2) for detecting/retrieving mineral dust aerosol. A methodology for separating dust from clouds and retrieving the dust IR optical depths was developed by exploiting differences between their spectral absorptive powers in prescribed thermal IR window subbands. Dust microphysical models were constructed using in situ data from the UAE2 and prior field studies while composition was modeled using refractive index data sets for minerals commonly observed around the UAE region including quartz, kaolinite, and calcium carbonate. The T-matrix, finite difference time domain (FDTD), and Lorenz-Mie light scattering programs were employed to calculate the single scattering properties for three dust shapes: oblate spheroids, hexagonal plates, and spheres. We used the Code for High-resolution Accelerated Radiative Transfer with Scattering (CHARTS) radiative transfer program to investigate sensitivity of the modeled AERI spectra to key dust and atmospheric parameters. Sensitivity studies show that characterization of the thermodynamic boundary layer is crucial for accurate AERI dust detection/retrieval. Furthermore, AERI sensitivity to dust optical depth is manifested in the strong subband slope dependence of the window region. Two daytime UAE2 cases were examined to demonstrate the present detection/retrieval technique, and we show that the results compare reasonably well to collocated AERONET Sun photometer/MPLNET micropulse lidar measurements. Finally, sensitivity of the developed methodology to the AERI's estimated MgCdTe detector nonlinearity was evaluated.

  17. Characterization and radiative impact of dust aerosols over northwestern part of India: a case study during a severe dust storm

    NASA Astrophysics Data System (ADS)

    Singh, Atinderpal; Tiwari, Shani; Sharma, Deepti; Singh, Darshan; Tiwari, Suresh; Srivastava, Atul Kumar; Rastogi, Neeraj; Singh, A. K.

    2016-12-01

    The present study focused on examining the impact of a severe dust storm (DS) on aerosol properties over Patiala (30.33°N, 76.4°E), a site located in the northwestern part of India during 20th-23rd March, 2012. On 20th March, average PM10 mass concentration increased abruptly from 182 to 817 µg m-3 along with significant increase in the number density of coarser particles (diameter >0.45 µm). During DS, spectral aerosol optical depth (AOD) increases significantly with more increase at longer wavelengths resulting in weak wavelength dependence (AOD at 380 nm increases by 210 % and at 870 nm by 270 % on 20th March). Significant decrease in Ångström exponent (AE; α 380-870) from 0.56 to 0.11 and fine-mode fraction (FMF; PM2.5/PM10) from 0.49 to 0.25 indicates dominance of coarser particles over the station. Net short wave (SW) radiation flux has been decreased by 20 % and single scattering albedo (SSA675) has been increased from 0.86 (19th March) to 0.90 (20th March). This observation is attributed to additional loading of scattering type aerosols on arrival of DS. Wavelength dependence of SSA reverses during DS and it increases with wavelength due to dominance of coarse-mode particles. Atmospheric aerosol radiative forcing (ATM ARF) during DS ranged from +45 to +77 W m-2, consequently heating the lower atmosphere up to 2.2 K day-1. Significant atmospheric heating rate due to severe dust storm may affect the regional atmospheric dynamics and hence the climate system.

  18. An Evaluation of Sharp Cut Cyclones for Sampling Diesel Particulate Matter Aerosol in the Presence of Respirable Dust

    PubMed Central

    Cauda, Emanuele; Sheehan, Maura; Gussman, Robert; Kenny, Lee; Volkwein, Jon

    2015-01-01

    Two prototype cyclones were the subjects of a comparative research campaign with a diesel particulate matter sampler (DPMS) that consists of a respirable cyclone combined with a downstream impactor. The DPMS is currently used in mining environments to separate dust from the diesel particulate matter and to avoid interferences in the analysis of integrated samples and direct-reading monitoring in occupational environments. The sampling characteristics of all three devices were compared using ammonium fluorescein, diesel, and coal dust aerosols. With solid spherical test aerosols at low particle loadings, the aerodynamic size-selection characteristics of all three devices were found to be similar, with 50% penetration efficiencies (d50) close to the design value of 0.8 µm, as required by the US Mine Safety and Health Administration for monitoring occupational exposure to diesel particulate matter in US mining operations. The prototype cyclones were shown to have ‘sharp cut’ size-selection characteristics that equaled or exceeded the sharpness of the DPMS. The penetration of diesel aerosols was optimal for all three samplers, while the results of the tests with coal dust induced the exclusion of one of the prototypes from subsequent testing. The sampling characteristics of the remaining prototype sharp cut cyclone (SCC) and the DPMS were tested with different loading of coal dust. While the characteristics of the SCC remained constant, the deposited respirable coal dust particles altered the size-selection performance of the currently used sampler. This study demonstrates that the SCC performed better overall than the DPMS. PMID:25060240

  19. Aerosol-Monsoon Interaction, maintenance and variability of the Asian Tropopause Aerosol Layer (ATAL)

    NASA Astrophysics Data System (ADS)

    Yuan, C.; Lau, W. K. M.; Li, Z.

    2016-12-01

    In recent years, the discovery of the Asian Tropopause Aerosol Layer (ATAL) from NASA satellite observations has sparked much interests in research on its composition, origin and relationships to the transport processes of atmospheric constituents in the upper troposphere and lower stratosphere (UTLS) and the variability of the Asian Monsoon Anticyclone (AMA). In this paper, based on analysis of MERRA2 reanalysis data, we present results showing that: 1) water vapor, aerosols and chemical gases (BC, OC, dust and CO) originated for the earth surface contribute significantly to the composition of the ATAL during the Asian summer monsoon, 2) one of the major pathways is via the strong large-scale vertical motion, and convective ascent over the Northern Himalayan Foothills during the peak phase of the Indian monsoon, 3) once transported into the UTLS , atmospheric constituents are capped by the Tropopuase inversion Layer (TIL) and advected around within and in the vicinity of the AMA forming the ATAL, 4) the ATAL is modulated by UTLS transport processes which undergo intrinsic monsoon intraseasonal oscillations with 20-30 day quasi-periodicity, coupled to lower tropospheric monsoon dynamics and diabatic heating processes, 5) the pre-monsoon accumulation of absorbing aerosols (BC, OC and dust) over the Indo-Gangetic Plain is more than likely to play an important role in enhancing the UTLS transport of atmospheric constituents from the earth surface to the ATAL.

  20. Relations Between Cloud Condensation Nuclei And Aerosol Optical Properties Relevant to Remote Sensing: Airborne Measurements in Biomass Burning, Pollution and Dust Aerosol Over North America

    NASA Astrophysics Data System (ADS)

    Shinozuka, Y.; Clarke, A.; Howell, S.; Kapustin, V.; McNaughton, C.; Zhou, J.; Decarlo, P.; Jimenez, J.; Roberts, G.; Tomlinson, J.; Collins, D.

    2008-12-01

    Remote sensing of the concentration of cloud condensation nuclei (CCN) would help investigate the indirect effect of tropospheric aerosols on clouds and climate. In order to assess its feasibility, this paper evaluates the spectral-based retrieval technique for aerosol number and seeks one for aerosol solubility, using in-situ aircraft measurements of aerosol size distribution, chemical composition, hygroscopicity, CCN activity and optical properties. Our statistical analysis reveals that the CCN concentration over Mexico can be optically determined to a relative error of <20%, smaller than that for the mainland US and the surrounding oceans (~a factor of 2). Mexico's advantage is four-fold. Firstly, many particles originating from the lightly regulated industrial combustion and biomass burning are large enough to significantly affect light extinction, elevating the correlation between extinction and CCN number in absence of substantial dust. Secondly, the generally low ambient humidity near the major aerosol sources limits the error in the estimated response of particle extinction to humidity changes. Thirdly, because many CCN contain black carbon, light absorption also provides a measure of the CCN concentration. Fourthly, the organic fraction of volatile mass of submicron particles (OMF) is anti-correlated with the wavelength dependence of extinction due to preferential anion uptake by coarse dust, which provides a potential tool for remote-sensing OMF and the particle solubility.

  1. Type-segregated aerosol effects on regional monsoon activity: A study using ground-based experiments and model simulations

    NASA Astrophysics Data System (ADS)

    Vijayakumar, K.; Devara, P. C. S.; Sonbawne, S. M.

    2014-12-01

    Classification of observed aerosols into key types [e.g., clean-maritime (CM), desert-dust (DD), urban-industrial/biomass-burning (UI/BB), black carbon (BC), organic carbon (OC) and mixed-type aerosols (MA)] would facilitate to infer aerosol sources, effects, and feedback mechanisms, not only to improve the accuracy of satellite retrievals but also to quantify the assessment of aerosol radiative impacts on climate. In this paper, we report the results of a study conducted in this direction, employing a Cimel Sun-sky radiometer at the Indian Institute of Tropical Meteorology (IITM), Pune, India during 2008 and 2009, which represent two successive contrasting monsoon years. The study provided an observational evidence to show that the local sources are subject to heavy loading of absorbing aerosols (dust and black carbon), with strong seasonality closely linked to the monsoon annual rainfall cycle over Pune, a tropical urban station in India. The results revealed the absence of CM aerosols in the pre-monsoon as well as in the monsoon seasons of 2009 as opposed to 2008. Higher loading of dust aerosols is observed in the pre-monsoon and monsoon seasons of 2009; majority may be coated with fine BC aerosols from local emissions, leading to reduction in regional rainfall. Further, significant decrease in coarse-mode AOD and presence of carbonaceous aerosols, affecting the aerosol-cloud interaction and monsoon-rain processes via microphysics and dynamics, is considered responsible for the reduction in rainfall during 2009. Additionally, we discuss how optical depth, contributed by different types of aerosols, influences the distribution of monsoon rainfall over an urban region using the Monitoring Atmospheric Composition and Climate (MACC) aerosol reanalysis. Furthermore, predictions of the Dust REgional Atmospheric Model (DREAM) simulations combined with HYSPLIT (HYbrid Single Particle Lagrangian Integrated Trajectory) cluster model are also discussed in support of the

  2. A study of remotely sensed aerosol properties from ground-based sun and sky scanning radiometers

    NASA Astrophysics Data System (ADS)

    Giles, David M.

    Aerosol particles impact human health by degrading air quality and affect climate by heating or cooling the atmosphere. The Indo-Gangetic Plain (IGP) of Northern India, one of the most populous regions in the world, produces and is impacted by a variety of aerosols including pollution, smoke, dust, and mixtures of them. The NASA Aerosol Robotic Network (AERONET) mesoscale distribution of Sun and sky-pointing instruments in India was established to measure aerosol characteristics at sites across the IGP and around Kanpur, India, a large urban and industrial center in the IGP, during the 2008 pre-monsoon (April-June). This study focused on detecting spatial and temporal variability of aerosols, validating satellite retrievals, and classifying the dominant aerosol mixing states and origins. The Kanpur region typically experiences high aerosol loading due to pollution and smoke during the winter and high aerosol loading due to the addition of dust to the pollution and smoke mixture during the pre-monsoon. Aerosol emissions in Kanpur likely contribute up to 20% of the aerosol loading during the pre-monsoon over the IGP. Aerosol absorption also increases significantly downwind of Kanpur indicating the possibility of the black carbon emissions from aerosol sources such as coal-fired power plants and brick kilns. Aerosol retrievals from satellite show a high bias when compared to the mesoscale distributed instruments around Kanpur during the pre-monsoon with few high quality retrievals due to imperfect aerosol type and land surface characteristic assumptions. Aerosol type classification using the aerosol absorption, size, and shape properties can identify dominant aerosol mixing states of absorbing dust and black carbon particles. Using 19 long-term AERONET sites near various aerosol source regions (Dust, Mixed, Urban/Industrial, and Biomass Burning), aerosol absorption property statistics are expanded upon and show significant differences when compared to previous work

  3. Reducing the Uncertainties in Direct Aerosol Radiative Forcing

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.

    2011-01-01

    Airborne particles, which include desert and soil dust, wildfire smoke, sea salt, volcanic ash, black carbon, natural and anthropogenic sulfate, nitrate, and organic aerosol, affect Earth's climate, in part by reflecting and absorbing sunlight. This paper reviews current status, and evaluates future prospects for reducing the uncertainty aerosols contribute to the energy budget of Earth, which at present represents a leading factor limiting the quality of climate predictions. Information from satellites is critical for this work, because they provide frequent, global coverage of the diverse and variable atmospheric aerosol load. Both aerosol amount and type must be determined. Satellites are very close to measuring aerosol amount at the level-of-accuracy needed, but aerosol type, especially how bright the airborne particles are, cannot be constrained adequately by current techniques. However, satellite instruments can map out aerosol air mass type, which is a qualitative classification rather than a quantitative measurement, and targeted suborbital measurements can provide the required particle property detail. So combining satellite and suborbital measurements, and then using this combination to constrain climate models, will produce a major advance in climate prediction.

  4. Towards a Global Aerosol Climatology: Preliminary Trends in Tropospheric Aerosol Amounts and Corresponding Impact on Radiative Forcing between 1950 and 1990

    NASA Technical Reports Server (NTRS)

    Tegen, Ina; Koch, Dorothy; Lacis, Andrew A.; Sato, Makiko

    1999-01-01

    A global aerosol climatology is needed in the study of decadal temperature change due to natural and anthropogenic forcing of global climate change. A preliminary aerosol climatology has been developed from global transport models for a mixture of sulfate and carbonaceous aerosols from fossil fuel burning, including also contributions from other major aerosol types such as soil dust and sea salt. The aerosol distributions change for the period of 1950 to 1990 due to changes in emissions of SO2 and carbon particles from fossil fuel burning. The optical thickness of fossil fuel derived aerosols increased by nearly a factor of 3 during this period, with particularly strong increase in eastern Asia over the whole time period. In countries where environmental laws came into effect since the early 1980s (e.g. US and western Europe), emissions and consequently aerosol optical thicknesses did not increase considerably after 1980, resulting in a shift in the global distribution pattern over this period. In addition to the optical thickness, aerosol single scattering albedos may have changed during this period due to different trends in absorbing black carbon and reflecting sulfate aerosols. However, due to the uncertainties in the emission trends, this change cannot be determined with any confidence. Radiative forcing of this aerosol distribution is calculated for several scenarios, resulting in a wide range of uncertainties for top-of-atmosphere (TOA) forcings. Uncertainties in the contribution of the strongly absorbing black carbon aerosol leads to a range in TOA forcings of ca. -0.5 to + 0.1 Wm (exp. -2), while the change in aerosol distributions between 1950 to 1990 leads to a change of -0.1 to -0.3 Wm (exp. -2), for fossil fuel derived aerosol with a "moderate" contribution of black carbon aerosol.

  5. Chemical Composition Characteristics of Atmospheric Aerosols in Relation to Haze, Asian Dust and Mixed Haze-Asian Dust Episodes at Background Site of Korea in 2013

    NASA Astrophysics Data System (ADS)

    KO, H.; Song, J. M.; Cha, J. W.; Kang, C. H.; Kim, J.; Ryoo, S. B.

    2016-12-01

    The PM10 and PM2.5 aerosols were collected at the Gosan site of Jeju Island, Korea in 2013 and analyzed, in order to examine the variation characteristics of chemical compositions in relation to haze, Asian dust, and mixed haze-Asian dust episodes. For the haze event, nitrate concentrations increased highly as 8.8 and 25.1 times for PM10 and PM2.5, respectively, possibly caused by the inflow of air mass stagnated in eastern parts of China into Jeju area. For the Asian dust event, the concentrations of nss-Ca2+, NO3- and nss-SO42- increased 6.0, 1.5, 1.8 times for PM10, and 2.3, 1.3, 1.6 times for PM2.5, respectively. Meanwhile, for the mixed haze-Asian dust event, the concentrations of nss-Ca2+ and NO3- increased 13.4 and 3.2 times for PM10, and 1.8 and 3.4 times for PM2.5, respectively. The NH4NO3 content was higher than that of (NH4)2SO4 during the haze event, however it was relatively low during the mixed haze-Asian dust event. NO3-/nss-SO42- concentration ratios of Asian Dust in PM10 and PM2.5 were 0.4 and 0.2, showing less significant effect from automobile and local pollution sources. The aerosols were acidified mostly by inorganic acids, especially the nitric acid contributed highly to the acidification during both haze and mixed haze-Asian dust events. Meanwhile, the neutralization by ammonia was noticeably high during haze event when the stagnated air mass moved from China.

  6. Ice nucleation activity of agricultural soil dust aerosols from Mongolia, Argentina, and Germany

    NASA Astrophysics Data System (ADS)

    Steinke, I.; Funk, R.; Busse, J.; Iturri, A.; Kirchen, S.; Leue, M.; Möhler, O.; Schwartz, T.; Schnaiter, M.; Sierau, B.; Toprak, E.; Ullrich, R.; Ulrich, A.; Hoose, C.; Leisner, T.

    2016-11-01

    Soil dust particles emitted from agricultural areas contain considerable mass fractions of organic material. Also, soil dust particles may act as carriers for potentially ice-active biological particles. In this work, we present ice nucleation experiments conducted in the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) cloud chamber. We investigated the ice nucleation efficiency of four types of soil dust from different regions of the world. The results are expressed as ice nucleation active surface site (INAS) densities and presented for the immersion freezing and the deposition nucleation mode. For immersion freezing occurring at 254 K, samples from Argentina, China, and Germany show ice nucleation efficiencies which are by a factor of 10 higher than desert dusts. On average, the difference in ice nucleation efficiencies between agricultural and desert dusts becomes significantly smaller at temperatures below 247 K. In the deposition mode the soil dusts showed higher ice nucleation activity than Arizona Test Dust over a temperature range between 232 and 248 K and humidities RHice up to 125%. INAS densities varied between 109 and 1011 m-2 for these thermodynamic conditions. For one soil dust sample (Argentinian Soil), the effect of treatments with heat was investigated. Heat treatments (383 K) did not affect the ice nucleation efficiency observed at 249 K. This finding presumably excludes proteinaceous ice-nucleating entities as the only source of the increased ice nucleation efficiency.

  7. MISR Global Aerosol Product Assessment by Comparison with AERONET

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.; Gaitley, Barbara J.; Garay, Michael J.; Diner, David J.; Eck, Thomas F.; Smirnov, Alexander; Holben, Brent N.

    2010-01-01

    A statistical approach is used to assess the quality of the MISR Version 22 (V22) aerosol products. Aerosol Optical Depth (AOD) retrieval results are improved relative to the early post- launch values reported by Kahn et al. [2005a], varying with particle type category. Overall, about 70% to 75% of MISR AOD retrievals fall within 0.05 or 20% AOD of the paired validation data, and about 50% to 55% are within 0.03 or 10% AOD, except at sites where dust, or mixed dust and smoke, are commonly found. Retrieved particle microphysical properties amount to categorical values, such as three groupings in size: "small," "medium," and "large." For particle size, ground-based AERONET sun photometer Angstrom Exponents are used to assess statistically the corresponding MISR values, which are interpreted in terms of retrieved size categories. Coincident Single-Scattering Albedo (SSA) and fraction AOD spherical data are too limited for statistical validation. V22 distinguishes two or three size bins, depending on aerosol type, and about two bins in SSA (absorbing vs. non-absorbing), as well as spherical vs. non-spherical particles, under good retrieval conditions. Particle type sensitivity varies considerably with conditions, and is diminished for mid-visible AOD below about 0.15 or 0.2. Based on these results, specific algorithm upgrades are proposed, and are being investigated by the MISR team for possible implementation in future versions of the product.

  8. Impacts of solar-absorbing aerosol layers on the transition of stratocumulus to trade cumulus clouds

    NASA Astrophysics Data System (ADS)

    Zhou, Xiaoli; Ackerman, Andrew S.; Fridlind, Ann M.; Wood, Robert; Kollias, Pavlos

    2017-10-01

    The effects of an initially overlying layer of solar-absorbing aerosol on the transition of stratocumulus to trade cumulus clouds are examined using large-eddy simulations. For lightly drizzling cloud the transition is generally hastened, resulting mainly from increased cloud droplet number concentration (Nc) induced by entrained aerosol. The increased Nc slows sedimentation of cloud droplets and shortens their relaxation time for diffusional growth, both of which accelerate entrainment of overlying air and thereby stratocumulus breakup. However, the decrease in albedo from cloud breakup is more than offset by redistributing cloud water over a greater number of droplets, such that the diurnal-average shortwave forcing at the top of the atmosphere is negative. The negative radiative forcing is enhanced by sizable longwave contributions, which result from the greater cloud breakup and a reduced boundary layer height associated with aerosol heating. A perturbation of moisture instead of aerosol aloft leads to a greater liquid water path and a more gradual transition. Adding absorbing aerosol to that atmosphere results in substantial reductions in liquid water path (LWP) and cloud cover that lead to positive shortwave and negative longwave forcings on average canceling each other. Only for heavily drizzling clouds is the breakup delayed, as inhibition of precipitation overcomes cloud water loss from enhanced entrainment. Considering these simulations as an imperfect proxy for biomass burning plumes influencing Namibian stratocumulus, we expect regional indirect plus semi-direct forcings to be substantially negative to negligible at the top of the atmosphere, with its magnitude sensitive to background and perturbation properties.

  9. Impacts of Solar-Absorbing Aerosol Layers on the Transition of Stratocumulus to Trade Cumulus Clouds

    NASA Technical Reports Server (NTRS)

    Zhou, Xiaoli; Ackerman, Andrew S.; Fridlind, Ann M.; Wood, Robert; Kollias, Pavlos

    2017-01-01

    The effects of an initially overlying layer of solar-absorbing aerosol on the transition of stratocumulus to trade cumulus clouds are examined using large-eddy simulations. For lightly drizzling cloud the transition is generally hastened, resulting mainly from increased cloud droplet number concentration (Nc) induced by entrained aerosol. The increased Nc slows sedimentation of cloud droplets and shortens their relaxation time for diffusional growth, both of which accelerate entrainment of overlying air and thereby stratocumulus breakup. However, the decrease in albedo from cloud breakup is more than offset by redistributing cloud water over a greater number of droplets, such that the diurnal-average shortwave forcing at the top of the atmosphere is negative. The negative radiative forcing is enhanced by sizable longwave contributions, which result from the greater cloud breakup and a reduced boundary layer height associated with aerosol heating. A perturbation of moisture instead of aerosol aloft leads to a greater liquid water path and a more gradual transition. Adding absorbing aerosol to that atmosphere results in substantial reductions in liquid water path (LWP) and cloud cover that lead to positive short-wave and negative longwave forcings on average canceling each other. Only for heavily drizzling clouds is the breakup delayed, as inhibition of precipitation overcomes cloud water loss from enhanced entrainment. Considering these simulations as an imperfect proxy for biomass burning plumes influencing Namibian stratocumulus, we expect regional indirect plus semi-direct forcings to be substantially negative to negligible at the top of the atmosphere, with its magnitude sensitive to background and perturbation properties.

  10. Three-dimensional variational assimilation of MODIS aerosol optical depth: Implementation and application to a dust storm over East Asia

    NASA Astrophysics Data System (ADS)

    Liu, Zhiquan; Liu, Quanhua; Lin, Hui-Chuan; Schwartz, Craig S.; Lee, Yen-Huei; Wang, Tijian

    2011-12-01

    Assimilation of the Moderate Resolution Imaging Spectroradiometer (MODIS) total aerosol optical depth (AOD) retrieval products (at 550 nm wavelength) from both Terra and Aqua satellites have been developed within the National Centers for Environmental Prediction (NCEP) Gridpoint Statistical Interpolation (GSI) three-dimensional variational (3DVAR) data assimilation system. This newly developed algorithm allows, in a one-step procedure, the analysis of 3-D mass concentration of 14 aerosol variables from the Goddard Chemistry Aerosol Radiation and Transport (GOCART) module. The Community Radiative Transfer Model (CRTM) was extended to calculate AOD using GOCART aerosol variables as input. Both the AOD forward model and corresponding Jacobian model were developed within the CRTM and used in the 3DVAR minimization algorithm to compute the AOD cost function and its gradient with respect to 3-D aerosol mass concentration. The impact of MODIS AOD data assimilation was demonstrated by application to a dust storm from 17 to 24 March 2010 over East Asia. The aerosol analyses initialized Weather Research and Forecasting/Chemistry (WRF/Chem) model forecasts. Results indicate that assimilating MODIS AOD substantially improves aerosol analyses and subsequent forecasts when compared to MODIS AOD, independent AOD observations from the Aerosol Robotic Network (AERONET) and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument, and surface PM10 (particulate matter with diameters less than 10 μm) observations. The newly developed AOD data assimilation system can serve as a tool to improve simulations of dust storms and general air quality analyses and forecasts.

  11. Ground level and Lidar monitoring of volcanic dust and dust from Patagonia

    NASA Astrophysics Data System (ADS)

    Otero, L. A.; Losno, R.; Salvador, J. O.; Journet, E.; Qu, Z.; Triquet, S.; Monna, F.; Balkanski, Y.; Bulnes, D.; Ristori, P. R.; Quel, E. J.

    2013-05-01

    A combined approach including ground level aerosol sampling, lidar and sunphotometer measurements is used to monitor suspended particles in the atmosphere at several sites in Patagonia. Motivated by the Puyehue volcanic eruption in June 2011 two aerosol monitoring stations with several passive and active instruments were installed in Bariloche and Comodoro Rivadavia. The main goal which is to monitor ground lifted and transported ashes and dust involving danger to civil aviation, is achieved by measuring continuously aerosol concentration at ground level and aerosol vertical distribution using lidar. In addition, starting from December 2011, continuous series of weekly accumulated aerosol concentrations at Rio Gallegos are being measured to study the impact of Patagonian dust over the open ocean on phytoplankton primary productivity and CO2 removal. These measurements are going to be coupled with LIDAR monitoring and a dust optical response models to test if aerosol extrapolation can be done from the ground to the top of the layer. Laboratory chemical analysis of the aerosols will include elemental composition, solubilisation kinetic and mineralogical determination. Expected deliverables for this study is the estimation of the amount of dust exported from Patagonia towards the South Atlantic, its chemical properties, including bioavailability simulation, from model and comparison to experimental measurements.

  12. Comparison of mineral dust and droplet residuals measured with two single particle aerosol mass spectrometers

    NASA Astrophysics Data System (ADS)

    Wonaschütz, Anna; Ludwig, Wolfgang; Zawadowicz, Maria; Hiranuma, Naruki; Hitzenberger, Regina; Cziczo, Daniel; DeMott, Paul; Möhler, Ottmar

    2017-04-01

    Single Particle mass spectrometers are used to gain information on the chemical composition of individual aerosol particles, aerosol mixing state, and other valuable aerosol characteristics. During the Mass Spectrometry Intercomparison at the Fifth Ice Nucleation (FIN-01) Workshop, the new LAAPTOF single particle aerosol mass spectrometer (AeroMegt GmbH) was conducting simultaneous measurements together with the PALMS (Particle Analysis by Laser Mass Spectrometry) instrument. The aerosol particles were sampled from the AIDA chamber during ice cloud expansion experiments. Samples of mineral dust and ice droplet residuals were measured simultaneously. In this work, three expansion experiments are chosen for a comparison between the two mass spectrometers. A fuzzy clustering routine is used to group the spectra. Cluster centers describing the ensemble of particles are compared. First results show that while differences in the peak heights are likely due to the use of an amplifier in PALMS, cluster centers are comparable.

  13. Improving Aerosol Simulation over South Asia for Climate and Air Quality Studies

    NASA Technical Reports Server (NTRS)

    Pan, Xiaohua; Chin, Mian; Bian, Huisheng; Gautam, Ritesh

    2014-01-01

    Atmospheric pollution over South Asia attracts special attention due to its effects on regional climate, the water cycle, and human health. These effects are potentially growing owing to rising trends of anthropogenic aerosol emissions found there. However, it has been proved quite challenging to adequately represent the aerosol spatial distribution and magnitude over this critical region in global models (Pan et al. 2014), with the surface concentrations, aerosol optical depth (AOD), and absorbing AOD (AAOD) significantly underestimated, especially in October-January when the agricultural waste burning and anthropogenic aerosol dominate over dust aerosol. In this study, we aim to investigate the causes for such discrepancy in winter by conducting sets of model experiments with NASA's GEOS-5 in terms of (1) spatial resolution, (2) emission amount, and (3) meteorological fields.

  14. Top-down estimate of dust emissions through integration of MODIS and MISR aerosol retrievals with the GEOS-Chem adjoint model

    NASA Astrophysics Data System (ADS)

    Wang, Jun; Xu, Xiaoguang; Henze, Daven K.; Zeng, Jing; Ji, Qiang; Tsay, Si-Chee; Huang, Jianping

    2012-04-01

    Predicting the influences of dust on atmospheric composition, climate, and human health requires accurate knowledge of dust emissions, but large uncertainties persist in quantifying mineral sources. This study presents a new method for combined use of satellite-measured radiances and inverse modeling to spatially constrain the amount and location of dust emissions. The technique is illustrated with a case study in May 2008; the dust emissions in Taklimakan and Gobi deserts are spatially optimized using the GEOS-Chem chemical transport model and its adjoint constrained by aerosol optical depth (AOD) that are derived over the downwind dark-surface region in China from MODIS (Moderate Resolution Imaging Spectroradiometer) reflectance with the aerosol single scattering properties consistent with GEOS-chem. The adjoint inverse modeling yields an overall 51% decrease in prior dust emissions estimated by GEOS-Chem over the Taklimakan-Gobi area, with more significant reductions south of the Gobi Desert. The model simulation with optimized dust emissions shows much better agreement with independent observations from MISR (Multi-angle Imaging SpectroRadiometer) AOD and MODIS Deep Blue AOD over the dust source region and surface PM10 concentrations. The technique of this study can be applied to global multi-sensor remote sensing data for constraining dust emissions at various temporal and spatial scales, and hence improving the quantification of dust effects on climate, air quality, and human health.

  15. Top-down Estimate of Dust Emissions Through Integration of MODIS and MISR Aerosol Retrievals With the Geos-chem Adjoint Model

    NASA Technical Reports Server (NTRS)

    Wang, Jun; Xu, Xiaoguang; Henze, Daven K.; Zeng, Jing; Ji, Qiang; Tsay, Si-Chee; Huang, Jianping

    2012-01-01

    Predicting the influences of dust on atmospheric composition, climate, and human health requires accurate knowledge of dust emissions, but large uncertainties persist in quantifying mineral sources. This study presents a new method for combined use of satellite-measured radiances and inverse modeling to spatially constrain the amount and location of dust emissions. The technique is illustrated with a case study in May 2008; the dust emissions in Taklimakan and Gobi deserts are spatially optimized using the GEOSChem chemical transport model and its adjoint constrained by aerosol optical depth (AOD) that are derived over the downwind dark-surface region in China from MODIS (Moderate Resolution Imaging Spectroradiometer) reflectance with the aerosol single scattering properties consistent with GEOS-chem. The adjoint inverse modeling yields an overall 51% decrease in prior dust emissions estimated by GEOS-Chem over the Taklimakan-Gobi area, with more significant reductions south of the Gobi Desert. The model simulation with optimized dust emissions shows much better agreement with independent observations from MISR (Multi-angle Imaging SpectroRadiometer) AOD and MODIS Deep Blue AOD over the dust source region and surface PM10 concentrations. The technique of this study can be applied to global multi-sensor remote sensing data for constraining dust emissions at various temporal and spatial scales, and hence improving the quantification of dust effects on climate, air quality, and human health.

  16. Comparison of two different dust emission mechanisms over the Horqin Sandy Land area: Aerosols contribution and size distributions

    NASA Astrophysics Data System (ADS)

    Ju, Tingting; Li, Xiaolan; Zhang, Hongsheng; Cai, Xuhui; Song, Yu

    2018-03-01

    Dust aerosols (PM10) emission fluxes due to convective turbulent dust emissions (CTDE) and saltation-bombardment and/or aggregation-disintegration dust emissions (SADE) events were comparatively studied using the data obtained from the Naiman station over the Horqin Sandy Land area in Inner Mongolia, China from 2011 to 2015. The annual cumulative dust fluxes released by CTDE events was about one third of that by SADE events, with the order of 103∼104 μg m-2 s-1. The particle size distributions (PSDs) with diameter between 0.1 and 20 μm during CTDE and SADE events over the Horqin Sandy Land area were simulated based on the fragmentation theory, respectively. The results indicated that an improved equation based on fragmentation theory could be applied to describe the PSDs over the Horqin site which may be because the scale-invariant fragmentation theory mainly explains the PSDs of free dust particles on the surface, which differ from the PSDs of suspend airborne dust and the improved equation was more applicable to the PSDs of SADE events because the dust emission mechanism of SADE are saltation bombardment and aggregation disintegration. The number-related mean aerosol diameters (DN) barely varied under different friction velocity (u*) for SADE events, while the volume-related mean aerosol diameters (DV) changed distinctly with the change of u*. For CTDE events, the DN and DV had no obvious relationship with the change of u* because the dominating influence factor during CTDE event was thermal convection rather than u*. The mass-related PSDs usually exhibited a peak between 0.45 and 0.70 μm during SADE events, while for CTDE events there was a wide peak in the range of 0.10 0.70 μm. The results suggest that DN should be not be recommended as an individual parameter to describe the PSDs. The mass-related PSDs can effectively distinguish the SADE and CTDE events.

  17. Effects of mineral dust on global atmospheric nitrate concentrations

    NASA Astrophysics Data System (ADS)

    Karydis, V. A.; Tsimpidi, A. P.; Pozzer, A.; Astitha, M.; Lelieveld, J.

    2016-02-01

    This study assesses the chemical composition and global aerosol load of the major inorganic aerosol components, focusing on mineral dust and aerosol nitrate. The mineral dust aerosol components (i.e., Ca2+, Mg2+, K+, Na+) and their emissions are included in the ECHAM5/MESSy Atmospheric Chemistry model (EMAC). Gas/aerosol partitioning is simulated using the ISORROPIA-II thermodynamic equilibrium model that considers K+, Ca2+, Mg2+, NH4+, Na+, SO42-, NO3-, Cl-, and H2O aerosol components. Emissions of mineral dust are calculated online by taking into account the soil particle size distribution and chemical composition of different deserts worldwide. Presence of metallic ions can substantially affect the nitrate partitioning into the aerosol phase due to thermodynamic interactions. The model simulates highest fine aerosol nitrate concentration over urban and industrialized areas (1-3 µg m-3), while coarse aerosol nitrate is highest close to deserts (1-4 µg m-3). The influence of mineral dust on nitrate formation extends across southern Europe, western USA, and northeastern China. The tropospheric burden of aerosol nitrate increases by 44 % when considering interactions of nitrate with mineral dust. The calculated global average nitrate aerosol concentration near the surface increases by 36 %, while the coarse- and fine-mode concentrations of nitrate increase by 53 and 21 %, respectively. Other inorganic aerosol components are affected by reactive dust components as well (e.g., the tropospheric burden of chloride increases by 9 %, ammonium decreases by 41 %, and sulfate increases by 7 %). Sensitivity tests show that nitrate aerosol is most sensitive to the chemical composition of the emitted mineral dust, followed by the soil size distribution of dust particles, the magnitude of the mineral dust emissions, and the aerosol state assumption.

  18. CV-Dust: Atmospheric aerosol in the Cape Verde region: carbon and soluble fractions of PM10

    NASA Astrophysics Data System (ADS)

    Pio, C.; Nunes, T.; Cardoso, J.; Caseiro, A.; Custódio, D.; Cerqueira, M.; Patoilo, D.; Almeida, S. M.; Freitas, M. C.

    2012-04-01

    Every year, billions of tons of eroded mineral soils from the Saharan Desert and the Sahel region, the largest dust source in the world, cross Mediterranean towards Europe, western Asia and the tropical North Atlantic Ocean as far as the Caribbean and South America. Many aspects of the direct and indirect effects of dust on climate are not well understood and the bulk and surface chemistry of the mineral dust particles determines interactions with gaseous and other particle species. The quantification of the magnitude of warming or cooling remains open because of the strong variability of the atmospheric dust burden and the lack of representative data for the spatial and temporal distribution of the dust composition. CV-Dust is a project that aims at provide a detailed data on the size distribution and the size-resolved chemical and mineralogical composition of dust emitted from North Africa using a natural laboratory like Cape Verde. This archipelago is located in an area of massive dust transport from land to ocean, and is thus ideal to set up sampling devices that are able to characterize and quantify dust transported from Africa. Moreover, Cape Verde's future economic prospects depend heavily on the encouragement of tourism, therefore it is essential to elucidate the role of Saharan dust may play in the degradation of Cape Verde air quality. The main objectives of CV-Dust project are: 1) to characterize the chemical and mineralogical composition of dust transported from Africa by setting up an orchestra of aerosol sampling devices in the strategic archipelago of Cape Verde; 2) to identify the sources of particles in Cape Verde by using receptor models; 3) to elucidate the role Saharan dust may play in the degradation of Cape Verde air quality; 4) to model processes governing dust production, transport, interaction with the radiation field and removal from the atmosphere. Here we present part of the data obtained throughout the last year, involving a set of more

  19. The Impact of Atmospheric Aerosols on the Fraction of absorbed Photosynthetically Active Radiation

    NASA Astrophysics Data System (ADS)

    Veroustraete, Frank

    2010-05-01

    Aerosol pollution attracts a growing interest from atmospheric scientists with regard to their impact on health, the global climate and vegetation stress. A hypothesis, less investigated, is whether atmospheric aerosol interactions in the solar radiation field affect the amount of radiation absorbed by vegetation canopies and hence terrestrial vegetation productivity. Typically, aerosols affect vegetation canopy radiation absorption efficiency by altering the physical characteristics of solar radiation incoming on for example a forest canopy. It has been illustrated, that increasing mixing ratio's of atmospheric particulate matter lead to a higher fraction of diffuse sunlight as opposed to direct sunlight. It can be demonstrated, based on the application of atmospheric (MODTRAN) and leaf/canopy radiative transfer (LIBERTY/SPRINT) models, that radiation absorption efficiency in the PAR band of Picea like forests increases with increasing levels of diffuse radiation. It can be documented - on a theoretical basis - as well, that increasing aerosol loads in the atmosphere, induce and increased canopy PAR absorption efficiency. In this paper it is suggested, that atmospheric aerosols have to be taken into account when estimating vegetation gross primary productivity (GPP). The results suggest that Northern hemisphere vegetation CO2 uptake magnitude may increase with increasing atmospheric aerosol loads. Many climate impact scenario's related to vegetation productivity estimates, do not take this phenomenon into account. Boldly speaking, the results suggest a larger sink function for terrestrial vegetation than generally accepted. Keywords: Aerosols, vegetation, fAPAR, CO2 uptake, diffuse radiation.

  20. The role of mineral dust aerosols in polar amplification

    NASA Astrophysics Data System (ADS)

    Lambert, F.; Kug, J.; Park, R.; Jin, F.; Lee, J. H.

    2010-12-01

    During today’s global warming, as well as during glacial-interglacial changes, temperature increase is larger in polar areas than the global average, a phenomenon called “polar amplification”. Model studies suggest ice cap melting due to greenhouse gas induced temperature rise, and consequent decrease of albedo and enhanced oceanic and atmospheric heat transport, as the primary cause for this phenomenon in nowadays Arctic. However, the underlying causes for polar amplification on glacial-interglacial timescales are still unclear, especially in the Antarctic where sea ice coverage does not change as drastically as in the North. Recent results have shown that the temperature increase is not limited to the surface and that these changes can not be explained by snow and ice changes alone. Starting with dust flux measurements from ice cores in Greenland and Antarctica, we have estimated tropospheric concentrations using deposition velocities and vertical concentration profiles for Holocene and LGM conditions from the National Center for Atmospheric Research’s Community Climate System Model (CCSM3) and a 3-D global chemical transport model (GEOS-Chem). The radiative forcing due to mineral dust aerosols was then estimated using the GEOS-Chem model, based on the particle properties found in the ice. Preliminary results point towards positive forcing of dust because of the high albedo of the underlying ice sheets.

  1. Estimation of Asian Dust Aerosol Effect on Cloud Radiation Forcing Using Fu-Liou Radiative Model and CERES Measurements

    NASA Technical Reports Server (NTRS)

    Su, Jing; Huang, Jianping; Fu, Qiang; Minnis, Patrick; Ge, Jinming; Bi, Jianrong

    2008-01-01

    The impact of Asian dust on cloud radiative forcing during 2003-2006 is studied by using the Earth's Radiant Energy Budget Scanner (CERES) data and the Fu-Liou radiative transfer model. Analysis of satellite data shows that the dust aerosol significantly reduced the cloud cooling effect at TOA. In dust contaminated cloudy regions, the 4-year mean values of the instantaneous shortwave, longwave and net cloud radiative forcing are -138.9, 69.1, and -69.7 Wm(sup -2), which are 57.0, 74.2, and 46.3%, respectively, of the corresponding values in more pristine cloudy regions. The satellite-retrieved cloud properties are significantly different in the dusty regions and can influence the radiative forcing indirectly. The contributions to the cloud radiation forcing by the dust direct, indirect and semi-direct effects are estimated using combined satellite observations and Fu-Liou model simulation. The 4-year mean value of combination of indirect and semi-direct shortwave radiative forcing (SWRF) is 82.2 Wm(sup -2), which is 78.4% of the total dust effect. The direct effect is only 22.7 Wm(sup -2), which is 21.6% of the total effect. Because both first and second indirect effects enhance cloud cooling, the aerosol-induced cloud warming is mainly the result of the semi-direct effect of dust.

  2. An 11-year analysis of satellite retrievals of dust aerosol over the Red Sea and the Persian Gulf

    NASA Astrophysics Data System (ADS)

    Banks, Jamie; Brindley, Helen; Schepanski, Kerstin; Stenchikov, Georgiy

    2017-04-01

    As enclosed seas bordering two large desert regions, the Saharan and Arabian deserts, the maritime environments of the Red Sea and the Persian Gulf are heavily influenced by the presence of desert dust aerosol. The inter-annual variability of dust presence over the Red Sea is analysed and presented, with respect to the summer-time latitudinal gradient in dust loading, which is at a maximum in the far south of the Red Sea and at a minimum in the far north. Two satellite aerosol optical depth (AOD) products from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) and the MODerate resolution Imaging Spectroradiometer (MODIS) instruments are used to quantify this loading over the region. Over an eleven-year period from 2005-2015 the July mean SEVIRI AODs at 630 nm vary between 0.48 and 1.45 in the southern half of the Sea, while in the north this varies between 0.22 and 0.66. Inter-retrieval offsets are observed to occur at higher dust loadings, with pronounced positive MODIS-SEVIRI AOD offsets at AODs greater than 1, indicating substantial and systematic differences between the retrievals over the Red Sea at high dust loadings. These differences appear to be influenced in part by the differences in scattering angle range of the satellite measurements, implying that assumptions of particle shape introduce more substantial biases at the highest dust loadings.

  3. Study of atmospheric scattering and absorbing aerosols at 550 nm over nearby western Indian tropical sites of Thar Desert effected region

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Vyas, B. M., E-mail: bmvyas@yahoo.com; Saxenna, Abhishek; Panwar, Chhagan

    The first time experimental results based on spaced satellite observations of different kinds of aerosols properties have been described over two different contrast environmental conditions locations in western tropical Indian region specifically first at Jaisalmer (26.90°N, 69.90°E, 220 m above mean sea level (amsl)) located in central Thar dessert vicinity of western Indian site over Indian Thar Desert region and another at Udaipur (24.6° N, 73.7° E, 560 m amsl) site concerning to semi-urban and semi arid place of hilly areas. The daily values of aerosols optical depth absorption at 500nm (AOD abs 500nm), aerosols optical depth extinction at 500nmmore » (AOD ext 500nm) along with aerosols optical depth at 500nmon (AOD 500nm) of eleven year period from Jan., 2004 to Dec., 2014 are basis of primary database of the present investigation. From the synthesis if the above database and the basis of rigorous statistical approach, following some of interesting facts are noted (i) larger annual monthly AOD variation of 0.93 is noted over JSM when compared to observed annual monthly change in AOD cycle, over UDP, of only 0.50 clearly indicating the more impact of desert influence activities about more than double times over JSM than UDP (ii) The higher abundance of absorbing aerosols occurrences about two time higher are seen in JSM in comparison to UDP. It indicates the clear evidence of strong optical absorption properties of useful solar mid visible wavelength at 550nm as the results of presence of more availability of dust aerosols as mineral natural type in pre-monsoon to post-monsoon over JSM which is also more predominant over JSM than the UDP region located far away from desert activity regime (iii) The greater sharing of extinction solar radiation effect on aerosols are more effective in pre-monsoon in UDP in reference to over JSM, where as in case of UDP, the aerosols effect through the scattering mechanism gradually reduce from monsoon to winter months as

  4. PERSPECTIVE: Dust, fertilization and sources

    NASA Astrophysics Data System (ADS)

    Remer, Lorraine A.

    2006-11-01

    between a model and observations J. Geophys. Res. 111 D06207 (doi:10.1029/2005JD005791) [5] Ginoux P et al 2001 Sources and distribution of dust aerosol simulated with the GOCART model J. Geophys. Res. 106 20255-74 (doi:10.1029/2000JD000053) [6] Prospero J M, Ginoux P, Torres O, Nicholson S E and Gill T E 2002 Environmental characterization of global sources of atmospheric soil dust identified with the NIMBUS 7 total Ozone Mapping Spectrometer (TOMS) absorbing aerosol product Rev. Geophys. 40 (1) 1002 (doi:10.1029/2000RG000095) [7] Koren I, Kaufman Y J, Washington R, Todd M C, Rudich Y, Martins J V and Rosenfeld D 2006 The Bodélé depression: a single spot in the Sahara that provides most of the mineral dust to the Amazon forest Environ. Res Lett. 1 014005 (doi:10.1088/1748-9326/1/1/014005) Photo of Lorraine A Remer Lorraine A Remer received a BS degree in atmospheric science from the University of California, Davis, in 1980, an MS degree in oceanography from the Scripps Institution of Oceanography, University of California, San Diego, in 1983, and a PhD degree, also in atmospheric science from the University of California, Davis, in 1991. She became involved with the MODIS retrievals of atmospheric aerosols in 1991, first as a Research Scientist with Science Systems and Applications, Inc., and subsequently with the National Aeronautics and Space Administration, which she joined in 1998. She is an Associate Member of the MODIS Science Team and a Member of the Global Aerosol Climatology Project Science Team.

  5. Impact of Tropospheric Aerosol Absorption on Ozone Retrieval from buv Measurements

    NASA Technical Reports Server (NTRS)

    Torres, O.; Bhartia, P. K.

    1998-01-01

    The impact of tropospheric aerosols on the retrieval of column ozone amounts using spaceborne measurements of backscattered ultraviolet radiation is examined. Using radiative transfer calculations, we show that uv-absorbing desert dust may introduce errors as large as 10% in ozone column amount, depending on the aerosol layer height and optical depth. Smaller errors are produced by carbonaceous aerosols that result from biomass burning. Though the error is produced by complex interactions between ozone absorption (both stratospheric and tropospheric), aerosol scattering, and aerosol absorption, a surprisingly simple correction procedure reduces the error to about 1%, for a variety of aerosols and for a wide range of aerosol loading. Comparison of the corrected TOMS data with operational data indicates that though the zonal mean total ozone derived from TOMS are not significantly affected by these errors, localized affects in the tropics can be large enough to seriously affect the studies of tropospheric ozone that are currently undergoing using the TOMS data.

  6. Improvements to the OMI Near-uv Aerosol Algorithm Using A-train CALIOP and AIRS Observations

    NASA Technical Reports Server (NTRS)

    Torres, O.; Ahn, C.; Zhong, C.

    2014-01-01

    The height of desert dust and carbonaceous aerosols layers and, to a lesser extent, the difficulty in assessing the predominant size mode of these absorbing aerosol types, are sources of uncertainty in the retrieval of aerosol properties from near UV satellite observations. The availability of independent, near-simultaneous measurements of aerosol layer height, and aerosol-type related parameters derived from observations by other A-train sensors, makes possible the direct use of these parameters as input to the OMI (Ozone Monitoring Instrument) near UV retrieval algorithm. A monthly climatology of aerosol layer height derived from observations by the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) sensor, and real-time AIRS (Atmospheric Infrared Sounder) CO observations are used in an upgraded version of the OMI near UV aerosol algorithm. AIRS CO measurements are used as a reliable tracer of carbonaceous aerosols, which allows the identification of smoke layers in areas and times of the year where the dust-smoke differentiation is difficult in the near-UV. The use of CO measurements also enables the identification of elevated levels of boundary layer pollution undetectable by near UV observations alone. In this paper we discuss the combined use of OMI, CALIOP and AIRS observations for the characterization of aerosol properties, and show a significant improvement in OMI aerosol retrieval capabilities.

  7. Iceland Polar Vortex 2016 campaign: Winter and high-altitude dust size distributions with the balloon-borne Light Optical Aerosol Counter (LOAC)

    NASA Astrophysics Data System (ADS)

    Renard, Jean-Baptiste; Dagsson-Waldhauserova, Pavla; Olafsson, Haraldur; Arnalds, Olafur; Vignelles, Damien; Verdier, Nicolas

    2017-04-01

    Iceland has the largest area of volcaniclastic sandy desert on Earth where dust is originating from volcanic, but also glaciogenic sediments. Total Icelandic desert areas cover 44,000 km2 which makes Iceland the largest Arctic as well as European desert. The mean frequency of days with dust suspension was to 135 dust days annually in 1949-2011. The annual dust deposition was calculated as 31 - 40.1 million tons yr-1 affecting the area of > 500,000 km2. About 50% of the suspended PM10 are submicron particles. Icelandic dust is of volcanic origin; it is very dark in colour and contains sharp-tipped shards with bubbles. Such properties allow even large particles to be easily transported long distances as revealed on the satellite MODIS images with dust plumes traveling over 1000 km at times. There is a need to understand better the vertical distribution of such aerosols as well as their residence time in the atmosphere, especially during occasions such as polar vortex. Four LOAC flights were performed under meteorological balloons in Iceland in January 9-13 2016 when stratospheric polar vortex occurred above Iceland. LOAC is an optical aerosol counter that uses a new optical design to retrieve the size concentrations in 19 size classes between 0.2 and 100 micrometers, and to provide an estimate of the main nature of aerosols. Vertical profile of aerosol size distribution showed the presence of volcanic dust particles up to altitudes of 8 km for two of the flights (9-10 January). The MODIS satellite images confirmed a dust plume present above the southern coast from the deposits of September 2015 glacial outburst flood (jökulhlaup) while the rest of the country was covered by snow. These deposits had been actively suspended in November and December 2015. The ground PM10 mass concentration measurements in Reykjavik showed elevated PM measurements over 100 micrograms.m-3, confirming the particle presence 250 km far from the source. The number concentration exceeded 200

  8. Temporal variations in optical and microphysical properties of mineral dust and biomass burning aerosol derived from daytime Raman lidar observations over Warsaw, Poland

    NASA Astrophysics Data System (ADS)

    Janicka, Lucja; Stachlewska, Iwona S.; Veselovskii, Igor; Baars, Holger

    2017-11-01

    In July 2013, favorable weather conditions caused a severe events of advection of biomass burning particles of Canadian forest fires to Europe. The smoke layers were widely observed, especially in Western Europe. An unusual atmospheric aerosol composition was measured at the EARLINET site in Warsaw, Central Poland, during a short event that occurred between 11 and 21 UTC on 10th July 2013. Additionally to the smoke layer, mineral dust was detected in a separate layer. The long-range dust transport pathway followed an uncommon way; originating in Western Sahara, passing above middle Atlantic, and circulating over British Islands, prior to its arrival to Poland. An effective radius of 560 nm was obtained for Saharan dust over Warsaw. This relatively small effective radius is likely due to the long time of the transport. The aerosol-polarization-Raman PollyXT-UW lidar was used for a successful daytime Raman retrieval of the aerosol optical properties at selected times during this short event. The aerosol vertical structure during the inflow over Warsaw in terms of optical properties and depolarization was analyzed, indicating clear distinction of the layers. The microphysical properties were inverted from the lidar derived optical data for selected ranges as representing the smoke and the mineral dust. For smoke, the effective radius was in the range of 0.29-0.36 μm and the complex refractive index 1.36 + 0.008i, on average. For dust, the values of 0.33-0.56 μm and 1.56 + 0.004i were obtained. An evolution of the aerosol composition over Warsaw during the day was analyzed.

  9. Impacts of solar-absorbing aerosol layers on the transition of stratocumulus to trade cumulus clouds

    DOE PAGES

    Zhou, Xiaoli; Ackerman, Andrew S.; Fridlind, Ann M.; ...

    2017-10-26

    Here, the effects of an initially overlying layer of solar-absorbing aerosol on the transition of stratocumulus to trade cumulus clouds are examined using large-eddy simulations. For lightly drizzling cloud the transition is generally hastened, resulting mainly from increased cloud droplet number concentration ( N c) induced by entrained aerosol. The increased N c slows sedimentation of cloud droplets and shortens their relaxation time for diffusional growth, both of which accelerate entrainment of overlying air and thereby stratocumulus breakup. However, the decrease in albedo from cloud breakup is more than offset by redistributing cloud water over a greater number of droplets,more » such that the diurnal-average shortwave forcing at the top of the atmosphere is negative. The negative radiative forcing is enhanced by sizable longwave contributions, which result from the greater cloud breakup and a reduced boundary layer height associated with aerosol heating. A perturbation of moisture instead of aerosol aloft leads to a greater liquid water path and a more gradual transition. Adding absorbing aerosol to that atmosphere results in substantial reductions in liquid water path (LWP) and cloud cover that lead to positive shortwave and negative longwave forcings on average canceling each other. Only for heavily drizzling clouds is the breakup delayed, as inhibition of precipitation overcomes cloud water loss from enhanced entrainment. Considering these simulations as an imperfect proxy for biomass burning plumes influencing Namibian stratocumulus, we expect regional indirect plus semi-direct forcings to be substantially negative to negligible at the top of the atmosphere, with its magnitude sensitive to background and perturbation properties.« less

  10. Impacts of solar-absorbing aerosol layers on the transition of stratocumulus to trade cumulus clouds

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Zhou, Xiaoli; Ackerman, Andrew S.; Fridlind, Ann M.

    Here, the effects of an initially overlying layer of solar-absorbing aerosol on the transition of stratocumulus to trade cumulus clouds are examined using large-eddy simulations. For lightly drizzling cloud the transition is generally hastened, resulting mainly from increased cloud droplet number concentration ( N c) induced by entrained aerosol. The increased N c slows sedimentation of cloud droplets and shortens their relaxation time for diffusional growth, both of which accelerate entrainment of overlying air and thereby stratocumulus breakup. However, the decrease in albedo from cloud breakup is more than offset by redistributing cloud water over a greater number of droplets,more » such that the diurnal-average shortwave forcing at the top of the atmosphere is negative. The negative radiative forcing is enhanced by sizable longwave contributions, which result from the greater cloud breakup and a reduced boundary layer height associated with aerosol heating. A perturbation of moisture instead of aerosol aloft leads to a greater liquid water path and a more gradual transition. Adding absorbing aerosol to that atmosphere results in substantial reductions in liquid water path (LWP) and cloud cover that lead to positive shortwave and negative longwave forcings on average canceling each other. Only for heavily drizzling clouds is the breakup delayed, as inhibition of precipitation overcomes cloud water loss from enhanced entrainment. Considering these simulations as an imperfect proxy for biomass burning plumes influencing Namibian stratocumulus, we expect regional indirect plus semi-direct forcings to be substantially negative to negligible at the top of the atmosphere, with its magnitude sensitive to background and perturbation properties.« less

  11. Quantifying Above-Cloud Aerosols through Integrating Multi-Sensor Measurements from A-Train Satellites

    NASA Technical Reports Server (NTRS)

    Zhang, Yan

    2012-01-01

    Quantifying above-cloud aerosols can help improve the assessment of aerosol intercontinental transport and climate impacts. Large-scale measurements of aerosol above low-level clouds had been generally unexplored until very recently when CALIPSO lidar started to acquire aerosol and cloud profiles in June 2006. Despite CALIPSO s unique capability of measuring above-cloud aerosol optical depth (AOD), such observations are substantially limited in spatial coverage because of the lidar s near-zero swath. We developed an approach that integrates measurements from A-Train satellite sensors (including CALIPSO lidar, OMI, and MODIS) to extend CALIPSO above-cloud AOD observations to substantially larger areas. We first examine relationships between collocated CALIPSO above-cloud AOD and OMI absorbing aerosol index (AI, a qualitative measure of AOD for elevated dust and smoke aerosol) as a function of MODIS cloud optical depth (COD) by using 8-month data in the Saharan dust outflow and southwest African smoke outflow regions. The analysis shows that for a given cloud albedo, above-cloud AOD correlates positively with AI in a linear manner. We then apply the derived relationships with MODIS COD and OMI AI measurements to derive above-cloud AOD over the whole outflow regions. In this talk, we will present spatial and day-to-day variations of the above-cloud AOD and the estimated direct radiative forcing by the above-cloud aerosols.

  12. Spatial distribution of mineral dust single scattering albedo based on DREAM model

    NASA Astrophysics Data System (ADS)

    Kuzmanoski, Maja; Ničković, Slobodan; Ilić, Luka

    2016-04-01

    Mineral dust comprises a significant part of global aerosol burden. There is a large uncertainty in estimating role of dust in Earth's climate system, partly due to poor characterization of its optical properties. Single scattering albedo is one of key optical properties determining radiative effects of dust particles. While it depends on dust particle sizes, it is also strongly influenced by dust mineral composition, particularly the content of light-absorbing iron oxides and the mixing state (external or internal). However, an assumption of uniform dust composition is typically used in models. To better represent single scattering albedo in dust atmospheric models, required to increase accuracy of dust radiative effect estimates, it is necessary to include information on particle mineral content. In this study, we present the spatial distribution of dust single scattering albedo based on the Dust Regional Atmospheric Model (DREAM) with incorporated particle mineral composition. The domain of the model covers Northern Africa, Middle East and the European continent, with horizontal resolution set to 1/5°. It uses eight particle size bins within the 0.1-10 μm radius range. Focusing on dust episode of June 2010, we analyze dust single scattering albedo spatial distribution over the model domain, based on particle sizes and mineral composition from model output; we discuss changes in this optical property after long-range transport. Furthermore, we examine how the AERONET-derived aerosol properties respond to dust mineralogy. Finally we use AERONET data to evaluate model-based single scattering albedo. Acknowledgement We would like to thank the AERONET network and the principal investigators, as well as their staff, for establishing and maintaining the AERONET sites used in this work.

  13. Laboratory estimate of the regional shortwave refractive index and single scattering albedo of mineral dust from major sources worldwide

    NASA Astrophysics Data System (ADS)

    Di Biagio, C.; Formenti, P.; Caponi, L.; Cazaunau, M.; Pangui, E.; Journet, E.; Nowak, S.; Caquineau, S.; Andreae, M. O.; Kandler, K.; Saeed, T.; Piketh, S.; Seibert, D.; Williams, E.; Balkanski, Y.; Doussin, J. F.

    2017-12-01

    Mineral dust is one of the most abundant aerosol species in the atmosphere and strongly contributes to the global and regional direct radiative effect. Still large uncertainties persist on the magnitude and overall sign of the dust direct effect, where indeed one of the main unknowns is how much mineral dust absorbs light in the shortwave (SW) spectral range. Aerosol absorption is represented both by the imaginary part (k) of the complex refractive index or the single scattering albedo (SSA, i.e. the ratio of the scattering to extinction coefficient). In this study we present a new dataset of SW complex refractive indices and SSA for mineral dust aerosols obtained from in situ measurements in the 4.2 m3 CESAM simulation chamber at LISA (Laboratoire Interuniversitaire des Systemes Atmospheriques) in Créteil, France. Investigated dust aerosol samples were issued from major desert sources worldwide, including the African Sahara and Sahel, Eastern Asia, the Middle East, Southern Africa, Australia, and the Americas, with differing iron oxides content. Results from the present study provide a regional mapping of the SW absorption by dust and show that the imaginary part of the refractive index largely varies (by up to a factor 6, 0.003-0.02 at 370 nm and 0.001-0.003 at 950 nm) for the different source areas due to the change in the particle iron oxide content. The SSA for dust varies between 0.75-0.90 at 370 nm and 0.95-0.99 at 950 nm, with the largest absorption observed for Sahelian and Australian dust aerosols. Our range of variability for k and SSA is well bracketed by already published literature estimates, but suggests that regional‒dependent values should be used in models. The possible relationship between k and the dust iron oxides content is investigated with the aim of providing a parameterization of the regional‒dependent dust absorption to include in climate models.

  14. Evaluating the Assumptions of Surface Reflectance and Aerosol Type Selection Within the MODIS Aerosol Retrieval Over Land: The Problem of Dust Type Selection

    NASA Technical Reports Server (NTRS)

    Mielonen, T.; Levy, R. C.; Aaltonen, V.; Komppula, M.; de Leeuw, G.; Huttunen, J.; Lihavainen, H.; Kolmonen, P.; Lehtinen, K. E. J.; Arola, A.

    2011-01-01

    Aerosol Optical Depth (AOD) and Angstrom exponent (AE) values derived with the MODIS retrieval algorithm over land (Collection 5) are compared with ground based sun photometer measurements at eleven sites spanning the globe. Although, in general, total AOD compares well at these sites (R2 values generally over 0.8), there are cases (from 2 to 67% of the measurements depending on the site) where MODIS clearly retrieves the wrong spectral dependence, and hence, an unrealistic AE value. Some of these poor AE retrievals are due to the aerosol signal being too small (total AOD<0.3) but in other cases the AOD should have been high enough to derive accurate AE. However, in these cases, MODIS indicates AE values close to 0.6 and zero fine model weighting (FMW), i.e. dust model provides the best fitting to the MODIS observed reflectance. Yet, according to evidence from the collocated sun photometer measurements and back-trajectory analyses, there should be no dust present. This indicates that the assumptions about aerosol model and surface properties made by the MODIS algorithm may have been incorrect. Here we focus on problems related to parameterization of the land-surface optical properties in the algorithm, in particular the relationship between the surface reflectance at 660 and 2130 nm.

  15. Increasing aeolian dust deposition to snowpacks in the Rocky Mountains inferred from snowpack, wet deposition, and aerosol chemistry

    USGS Publications Warehouse

    Clow, David W.; Williams, Mark W.; Schuster, Paul F.

    2016-01-01

    Mountain snowpacks are a vital natural resource for ∼1.5 billion people in the northern Hemisphere, helping to meet human and ecological demand for water in excess of that provided by summer rain. Springtime warming and aeolian dust deposition accelerate snowmelt, increasing the risk of water shortages during late summer, when demand is greatest. While climate networks provide data that can be used to evaluate the effect of warming on snowpack resources, there are no established regional networks for monitoring aeolian dust deposition to snow. In this study, we test the hypothesis that chemistry of snow, wet deposition, and aerosols can be used as a surrogate for dust deposition to snow. We then analyze spatial patterns and temporal trends in inferred springtime dust deposition to snow across the Rocky Mountains, USA, for 1993–2014. Geochemical evidence, including strong correlations (r2 ≥ 0.94) between Ca2+, alkalinity, and dust concentrations in snow deposited during dust events, indicate that carbonate minerals in dust impart a strong chemical signature that can be used to track dust deposition to snow. Spatial patterns in chemistry of snow, wet deposition, and aerosols indicate that dust deposition increases from north to south in the Rocky Mountains, and temporal trends indicate that winter/spring dust deposition increased by 81% in the southern Rockies during 1993–2014. Using a multivariate modeling approach, we determined that increases in dust deposition and decreases in springtime snowfall combined to accelerate snowmelt timing in the southern Rockies by approximately 7–18 days between 1993 and 2014. Previous studies have shown that aeolian dust emissions may have doubled globally during the 20th century, possibly due to drought and land-use change. Climate projections for increased aridity in the southwestern U.S., northern Africa, and other mid-latitude regions of the northern Hemisphere suggest that aeolian dust emissions may continue to

  16. Constraining martian atmospheric dust particle size distributions from MER Navcam observations.

    NASA Astrophysics Data System (ADS)

    Soderblom, J. M.; Smith, M. D.

    2017-12-01

    Atmospheric dust plays an important role in atmospheric dynamics by absorbing energy and influencing the thermal structure of the atmosphere [1]. The efficiency by which dust absorbs energy depends on its size and single-scattering albedo. Characterizing these properties and their variability is, thus, important in modeling atmospheric circulation. Near-sun observations of the martian sky from Viking Lander, Mars Pathfinder, and MER Pancam images have been used to characterize the atmospheric scattering phase function. The forward-scattering peak the atmospheric phase function is primarily controlled by the size of aerosol particles and is less sensitive to atmospheric opacity or particle shape and single-scattering albedo [2]. These observations, however, have been limited to scattering angles >5°. We use the MER Navcams, which experience little-to-no debilitating internal instrumental scattered light during near-Sun imaging, enabling measurements of the brightness of the martian sky down to very small scattering angles [3], making them more sensitive to aerosol particle size. Additionally, the Navcams band-pass wavelength is similar to the dust effective particle size, further increasing this sensitivity. These data sample a wide range of atmospheric conditions, including variations in the atmospheric dust loading across the entire martian year, as well as more rapid variations during the onset and dissipation of a global-scale dust storm. General circulation models (GCMs) predict a size-dependence for the transport of dust during dust storms that would result in both spatial (on regional-to-global scales) and temporal (days-to-months) variations in the dust size distribution [4]. The absolute calibration of these data, however, is limited. The instrument temperature measurement is limited to a single thermocouple on the Opportunity left Navcam CCD, and observations of the calibration target by Navcam are infrequent. We discuss ways to mitigate these

  17. Aerosol and monsoon climate interactions over Asia

    NASA Astrophysics Data System (ADS)

    Li, Zhanqing; Lau, W. K.-M.; Ramanathan, V.; Wu, G.; Ding, Y.; Manoj, M. G.; Liu, J.; Qian, Y.; Li, J.; Zhou, T.; Fan, J.; Rosenfeld, D.; Ming, Y.; Wang, Y.; Huang, J.; Wang, B.; Xu, X.; Lee, S.-S.; Cribb, M.; Zhang, F.; Yang, X.; Zhao, C.; Takemura, T.; Wang, K.; Xia, X.; Yin, Y.; Zhang, H.; Guo, J.; Zhai, P. M.; Sugimoto, N.; Babu, S. S.; Brasseur, G. P.

    2016-12-01

    The increasing severity of droughts/floods and worsening air quality from increasing aerosols in Asia monsoon regions are the two gravest threats facing over 60% of the world population living in Asian monsoon regions. These dual threats have fueled a large body of research in the last decade on the roles of aerosols in impacting Asian monsoon weather and climate. This paper provides a comprehensive review of studies on Asian aerosols, monsoons, and their interactions. The Asian monsoon region is a primary source of emissions of diverse species of aerosols from both anthropogenic and natural origins. The distributions of aerosol loading are strongly influenced by distinct weather and climatic regimes, which are, in turn, modulated by aerosol effects. On a continental scale, aerosols reduce surface insolation and weaken the land-ocean thermal contrast, thus inhibiting the development of monsoons. Locally, aerosol radiative effects alter the thermodynamic stability and convective potential of the lower atmosphere leading to reduced temperatures, increased atmospheric stability, and weakened wind and atmospheric circulations. The atmospheric thermodynamic state, which determines the formation of clouds, convection, and precipitation, may also be altered by aerosols serving as cloud condensation nuclei or ice nuclei. Absorbing aerosols such as black carbon and desert dust in Asian monsoon regions may also induce dynamical feedback processes, leading to a strengthening of the early monsoon and affecting the subsequent evolution of the monsoon. Many mechanisms have been put forth regarding how aerosols modulate the amplitude, frequency, intensity, and phase of different monsoon climate variables. A wide range of theoretical, observational, and modeling findings on the Asian monsoon, aerosols, and their interactions are synthesized. A new paradigm is proposed on investigating aerosol-monsoon interactions, in which natural aerosols such as desert dust, black carbon from

  18. Improvement of Aerosol Optical Depth Retrieval from MODIS Spectral Reflectance over the Global Ocean Using New Aerosol Models Archived from AERONET Inversion Data and Tri-axial Ellipsoidal Dust Database

    NASA Technical Reports Server (NTRS)

    Lee, J.; Kim, J.; Yang, P.; Hsu, N. C.

    2012-01-01

    New over-ocean aerosol models are developed by integrating the inversion data from the Aerosol Robotic Network (AERONET) sun/sky radiometers with a database for the optical properties of tri-axial ellipsoid particles. The new aerosol models allow more accurate retrieval of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) in the case of high AOD (AOD greater than 0.3). The aerosol models are categorized by using the fine-mode fraction (FMF) at 550 nm and the singlescattering albedo (SSA) at 440 nm from the AERONET inversion data to include a variety of aerosol types found around the globe. For each aerosol model, the changes in the aerosol optical properties (AOPs) as functions of AOD are considered to better represent aerosol characteristics. Comparisons of AODs between AERONET and MODIS for the period from 2003 to 2010 show that the use of the new aerosol models enhances the AOD accuracy with a Pearson coefficient of 0.93 and a regression slope of 0.99 compared to 0.92 and 0.85 calculated using the MODIS Collection 5 data. Moreover, the percentage of data within an expected error of +/-(0.03 + 0.05xAOD) is increased from 62 percent to 64 percent for overall data and from 39 percent to 51 percent for AOD greater than 0.3. Errors in the retrieved AOD are further characterized with respect to the Angstrom exponent (AE), scattering angle, SSA, and air mass factor (AMF). Due to more realistic AOPs assumptions, the new algorithm generally reduces systematic errors in the retrieved AODs compared with the current operational algorithm. In particular, the underestimation of fine-dominated AOD and the scattering angle dependence of dust-dominated AOD are significantly mitigated as results of the new algorithm's improved treatment of aerosol size distribution and dust particle nonsphericity.

  19. The Effect of Asian Dust Aerosols on Cloud Properties and Radiative Forcing from MODIS and CERES

    NASA Technical Reports Server (NTRS)

    Huang, Jianping; Minnis, Patrick; Lin, Bing; Wang, Tianhe; Yi, Yuhong; Hu, Yongxiang; Sun-Mack, Sunny; Ayers, Kirk

    2005-01-01

    The effects of dust storms on cloud properties and radiative forcing are analyzed over northwestern China from April 2001 to June 2004 using data collected by the Moderate Resolution Imaging Spectroradiometer (MODIS) and Clouds and the Earth's Radiant Energy System (CERES) instruments on the Aqua and Terra satellites. On average, ice cloud effective particle diameter, optical depth and ice water path of the cirrus clouds under dust polluted conditions are 11%, 32.8%, and 42% less, respectively, than those derived from ice clouds in dust-free atmospheric environments. The humidity differences are larger in the dusty region than in the dust-free region, and may be caused by removal of moisture by wet dust precipitation. Due to changes in cloud microphysics, the instantaneous net radiative forcing is reduced from -71.2 W/m2 for dust contaminated clouds to -182.7 W/m2 for dust-free clouds. The reduced cooling effects of dusts may lead to a net warming of 1 W/m2, which, if confirmed, would be the strongest aerosol forcing during later winter and early spring dust storm seasons over the studied region.

  20. Characteristics of aerosol light scattering and absorption properties observed at Gosan, Korea, during GOPOEX 2014

    NASA Astrophysics Data System (ADS)

    Cho, C.; Kim, S. W.; Sheridan, P. J.; Gustafsson, O.; Lee, M.; Yoon, S. C.

    2016-12-01

    Anthropogenic fine pollution and wind-blown mineral dust aerosols have a significant effect on the regional radiation budget by scattering or absorbing the solar radiation reaching the Earth's surface. We investigate the optical and physical properties of dust and pollution aerosols at Gosan Climate Observatory (GCO), Korea during Gosan Pollution Experiment 2014 (GOPOEX 2014; January 2014).Mean values of aerosol scattering coefficient and absorption coefficient during GOPOEX 2014 were 72 ± 86 Mm-1 and 6 ± 5 Mm-1 at 550 nm, respectively. Aerosol scattering coefficient and absorption coefficient during dust episodes were 245 ± 171 Mm-1 and 22 ± 13 Mm-1 at 550 nm, which were approximately 3.5 times greater than mean values during GOPOEX 2014. Values for scattering and absorption coefficient of pollution episodes were recorded as 153 ± 95 Mm-1 and 12 ± 7 Mm-1 at 550 nm. Therefore, single scattering albedo of pollution episodes (0.92 ± 0.02) was slightly higher than those of dust episodes (0.90 ± 0.03). This is because that pollutant aerosols include more scattering fraction such as SO42-, and NO3- in fine particulate matter emitted from industrial areas in the eastern coastal region of China while dust aerosols are transported from North China to Gosan.Aerosol optical properties are influenced by where the air mass is transported from, either South China or North China. The mean values of aerosol scattering coefficient and absorption coefficient when air mass was transported from South China were 136 ± 132 Mm-1 and 15 ± 14 Mm-1 at 550 nm whereas those from North China were 108 ± 112 Mm-1 and 8 ± 7 Mm-1 at 550 nm. Single scattering albedo are almost identical as 0.9 ± 0.03 for both air masses.Carbonaceous composition of aerosols, which occupy a considerable fraction of fine particulate matter, also depends on the origin of the air mass. Radiocarbon (14C) is a good indicator for distinguishing between fossil combustion and biomass combustion. Detailed source

  1. Clear Sky Column Closure Studies of Urban-Marine and Mineral-Dust Aerosols Using Aircraft, Ship, Satellite and Ground-Based Measurements in ACE-2

    NASA Technical Reports Server (NTRS)

    Schmid, Beat; Russell, Philip B.; Livingston, John M.; Gasso, Santiago; Hegg, Dean A.; Collins, Donald R.; Flagan, Richard C.; Seinfeld, John H.; Oestroem, Elisabeth; Noone, Kevin J.; hide

    2000-01-01

    As part of the second Aerosol Characterization Experiment (ACE-2), European urban-marine and African mineral-dust aerosols were measured aboard the Pelican aircraft, the Research Vessel Vodyanitskiy from the ground and from satellites.

  2. Evaluation of applicability of high-resolution multiangle imaging photo-polarimetric observations for aerosol atmospheric correction

    NASA Astrophysics Data System (ADS)

    Kalashnikova, Olga; Garay, Michael; Xu, Feng; Diner, David; Seidel, Felix

    2016-07-01

    Multiangle spectro-polarimetric measurements have been advocated as an additional tool for better understanding and quantifying the aerosol properties needed for atmospheric correction for ocean color retrievals. The central concern of this work is the assessment of the effects of absorbing aerosol properties on remote sensing reflectance measurement uncertainty caused by neglecting UV-enhanced absorption of carbonaceous particles and by not accounting for dust nonsphericity. In addition, we evaluate the polarimetric sensitivity of absorbing aerosol properties in light of measurement uncertainties achievable for the next generation of multi-angle polarimetric imaging instruments, and demonstrate advantages and disadvantages of wavelength selection in the UV/VNIR range. In this work a vector Markov Chain radiative transfer code including bio-optical models was used to quantitatively evaluate in water leaving radiances between atmospheres containing realistic UV-enhanced and non-spherical aerosols and the SEADAS carbonaceous and dust-like aerosol models. The phase matrices for the spherical smoke particles were calculated using a standard Mie code, while those for non-spherical dust particles were calculated using the numerical approach developed for modeling dust for the AERONET network of ground-based sunphotometers. As a next step, we have developed a retrieval code that employs a coupled Markov Chain (MC) and adding/doubling radiative transfer method for joint retrieval of aerosol properties and water leaving radiance from Airborne Multiangle SpectroPolarimetric Imager-1 (AirMSPI-1) polarimetric observations. The AirMSPI-1 instrument has been flying aboard the NASA ER-2 high altitude aircraft since October 2010. AirMSPI typically acquires observations of a target area at 9 view angles between ±67° at 10 m resolution. AirMSPI spectral channels are centered at 355, 380, 445, 470, 555, 660, and 865 nm, with 470, 660, and 865 reporting linear polarization. We

  3. Light-absorbing aerosol properties retrieved from the sunphotometer observation over the Yangtze River Delta, China.

    PubMed

    Wang, Jing; Niu, Shengjie; Xu, Dan

    2018-02-10

    In this study, aerosol optical depth (AOD) and extinction Ångström exponent (EAE) are derived from ground-based sunphotometer observations between 2007 and 2014 at urban sites of Nanjing over the Yangtze River Delta. In addition, the present study aims to investigate aerosol light-absorbing properties such as single-scattering albedo (SSA), absorption Ångström exponent (AAE), and the aerosol-absorbing optical depth (AAOD). The retrieval of aerosol properties is compared with AERONET inversion products. The results demonstrate that the retrieved AOD has a good agreement with the AERONET Level 1.5 data, with the root mean square error being 0.068, 0.065, and 0.026 for total, fine mode, and coarse mode at 440 nm, respectively. The SSA values indicate similar accuracies in the results, which are about 0.003, -0.009, -0.008, and 0.010 different from AERONET at 440, 670, 870, and 1020 nm, respectively. The occurrence frequency of background level AOD (AOD<0.10) at 440 nm in this region is limited (1%). Monthly mean AOD, SSA, the effective radius (R eff ), and the volume concentration at 440 nm were 0.6-1.3, 0.85-0.92, 0.24-0.40 μm, and 0.18-0.28  μm 3  μm -2 , respectively. The mean value of AAOD at 440 nm (AAOD 440 ) was the highest in both summer (0.095±0.041) and autumn (0.094±0.042), but was the lowest in winter (0.079±0.036). It was also noted that SSA was found to be higher during summer (0.89±0.05). The spectral variation of SSA was observed to be strongly wavelength-dependent during all seasons. The seasonal mean AAE440-870 is the highest in winter (0.86±0.41) and lowest in spring (0.49±0.29). In winter, the cumulative frequency for AAE between 1.0 and 1.2 was about 87%. The peak in the AAE distribution was close to 1.0, indicating that the aerosol column was dominated by urban-industrial aerosols and absorption species other than black carbon. Analysis of the relationship between EAE and SSA showed that the aerosol populations could be

  4. Diagnosis of Dust- and Pollution- Impacted PM10, PM2.5, and PM1 Aerosols Observed at Gosan Climate Observatory

    NASA Astrophysics Data System (ADS)

    Shang, X.; Lee, M.; LIM, S.; Gustafsson, O.; Lee, G.; Chang, L.

    2017-12-01

    In East Asia, dust is prevalent and used to be mixed with various pollutants during transportation, causing a large uncertainty in estimating the climate forcing of aerosol and difficulty in making environmental policy. In order to diagnose the influence of dust particles on aerosol, we conducted a long-term measurement of PM10, PM2.5 and PM1 for mass, water-soluble ions, and carbonaceous compounds at Gosan Climate Observatory, South Korea from August 2007 to February 2012. The result of principle component analysis reveals that anthropogenic, typical soil dust, and saline dust impact explain 46 %, 16 %, and 9 % of the total variance for all samples, respectively. The mode analysis of mass distributions provides the criteria to distinguish these principle factors. The anthropogenic impact was most pronounced in PM1 and diagnosed by the PM1 mass higher than mean+σ. If PM10 mass was greater than mean+σ, it was highly likely to be affected by typical soil dust. This criterion is also applicable for PM2.5 mass, which was enhanced by both haze and dust particles, though. In the present study, saline dust was recognized by relatively high concentrations of Na and Cl ions in PM1.0. However, their existence was not manifested by increased mass in any of three PM types.

  5. Chemistry and Photochemistry at the Surface of Urban Road Dust and Photoactive Minerals

    NASA Astrophysics Data System (ADS)

    Styler, S. A.; Abou-Ghanem, M.; Wickware, B.

    2017-12-01

    Each year, over a billion tons of dust are released into the atmosphere from arid regions. After its emission, dust can undergo efficient long-range transport to urban centres, where it can interact with local pollution sources. Another source of dust in urban regions is road dust resuspension, which is the largest anthropogenic source of primary particulate matter in both Canada and the United States. Since dust contains light-absorbing components, including iron- and titanium-containing minerals, dust-catalyzed photochemical processes have the potential to influence both the lifetime of pollutants present at the dust surface and the composition of the surrounding atmosphere. To date, most studies of dust photochemistry have focused on TiO2-mediated processes, and no studies have explored trace gas uptake at the surface of road dust. Here, we present first results from aerosol and coated-wall flow tube investigations of ozone uptake at the surface of a suite of titanium-containing minerals and road dust collected in Edmonton, Alberta. Together, this work represents a significant advance in our understanding of chemistry and photochemistry at realistic environmental interfaces.

  6. Intercomparison of observations and model aerosol parameters during two Saharan dust events over the southern United Kingdom

    NASA Astrophysics Data System (ADS)

    Buxmann, Joelle; Adam, Mariana; Ordonez, Carlos; Tilbee, Marie; Smyth, Tim; Claxton, Bernard; Sugier, Jacqueline; Agnew, Paul

    2015-04-01

    Saharan desert dust lifted by convection over the hot desert surface can reach high altitudes and be transported over great distances. In the UK, Saharan dust episodes occur several times a year, usually during the spring. Dust lifted by cyclonic circulation is often blown into the Atlantic and transported to the UK. This can result in a rapid degradation of air quality due to the increase in the levels of particulate matter (PM). The ability to model the transport and deposition of dust remains an important challenge in order to characterize different pollution events. We present a comparison of observed Aerosol Optical Depth (AOD) with modelled AOD from the Met Office Air Quality Unified Model (AQUM), performed for two dust events in March 2014 (at 380nm, 440nm, 870nm and 1020nm). The observations are derived from five sun photometers located in the southern UK at Exeter, Cardington, Bayfordbury, Chilbolton, and Plymouth. Correlations are investigated between model column integrated PM2.5 and PM10, and observed fine and coarse mode AOD from AERONET. Vertical profiles of attenuated backscatter and extinction from the Jenoptik Nimbus ceilometers part of the Met Office Laser Cloud Base Recorder (LCBR) network are investigated as well (see also session AS3.17/GI2.2 Lidar and Applications). The Met Office air quality model AQUM is an on-line meteorology, chemistry and aerosol modelling system. It runs at a resolution of 12km over a domain covering the UK and north-western Europe. Atmospheric composition modelling employs two-way coupling between aerosol and chemistry evolution, with explicit modelling of sulphate, nitrate, black carbon, organic carbon, biomass burning and wind-blown mineral dust aerosol components. Both the model and observations show an increase in AOD during the first period from 12 -13 March 2014. For example AOD levels of up to 0.52 for the 380nm channel were recorded by the sun photometer in Exeter. This is relatively high compared to average

  7. Quantifying the response of the ORAC aerosol optical depth retrieval for MSG SEVIRI to aerosol model assumptions

    NASA Astrophysics Data System (ADS)

    Bulgin, Claire E.; Palmer, Paul I.; Merchant, Christopher J.; Siddans, Richard; Gonzi, Siegfried; Poulsen, Caroline A.; Thomas, Gareth E.; Sayer, Andrew M.; Carboni, Elisa; Grainger, Roy G.; Highwood, Eleanor J.; Ryder, Claire L.

    2011-03-01

    We test the response of the Oxford-RAL Aerosol and Cloud (ORAC) retrieval algorithm for Meteosat Second Generation Spinning Enhanced Visible and InfraRed Imager (MSG SEVIRI) to changes in the aerosol properties used in the dust aerosol model, using data from the Dust Outflow and Deposition to the Ocean (DODO) flight campaign in August 2006. We find that using the observed DODO free tropospheric aerosol size distribution and refractive index increases simulated top of the atmosphere radiance at 0.55 μm assuming a fixed aerosol optical depth of 0.5 by 10-15%, reaching a maximum difference at low solar zenith angles. We test the sensitivity of the retrieval to the vertical distribution of the aerosol and find that this is unimportant in determining simulated radiance at 0.55 μm. We also test the ability of the ORAC retrieval when used to produce the GlobAerosol data set to correctly identify continental aerosol outflow from the African continent, and we find that it poorly constrains aerosol speciation. We develop spatially and temporally resolved prior distributions of aerosols to inform the retrieval which incorporates five aerosol models: desert dust, maritime, biomass burning, urban, and continental. We use a Saharan Dust Index and the GEOS-Chem chemistry transport model to describe dust and biomass burning aerosol outflow and compare AOD using our speciation against the GlobAerosol retrieval during January and July 2006. We find AOD discrepancies of 0.2-1 over regions of intense biomass burning outflow, where AOD from our aerosol speciation and GlobAerosol speciation can differ by as much as 50-70%.

  8. In situ aerosol optics in Reno, NV, USA during and after the summer 2008 California wildfires and the influence of absorbing and non-absorbing organic coatings on spectral light absorption

    NASA Astrophysics Data System (ADS)

    Gyawali, M.; Arnott, W. P.; Lewis, K.; Moosmüller, H.

    2009-10-01

    Hundreds of wildfires in Northern California were sparked by lightning during the summer of 2008, resulting in downwind smoke for the months of June and July. Comparisons are reported for aerosol optics measurements in Reno, Nevada made during the very smoky month of July and the relatively clean month of August. Photoacoustic instruments equipped with integrating nephelometers were used to measure aerosol light scattering and absorption coefficients at wavelengths of 405 nm and 870 nm, revealing a strong variation of aerosol light absorption with wavelength. Insight on fuels burned is gleaned from comparison of Ångström exponents of absorption (AEA) versus single scattering albedo (SSA) of the ambient measurements with laboratory biomass smoke measurements for many fuels. Measurements during the month of August, which were largely unaffected by fire smoke, exhibit surprisingly low AEA for aerosol light absorption when the SSA is highest, again likely as a consequence of the underappreciated wavelength dependence of aerosol light absorption by particles coated with non-absorbing organic and inorganic matter. Coated sphere calculations were used to show that AEA as large as 1.6 are possible for wood smoke even with non-absorbing organic coatings on black carbon cores, suggesting care be exercised when diagnosing AEA.

  9. An Assessment of the Surface Longwave Direct Radiative Effect of Airborne Dust in Zhangye China During the Asian Monsoon Year Field Experiment (2008)

    NASA Technical Reports Server (NTRS)

    Hansell, Richard A.; Tsay, Si-Chee; Hsu, N. Christina; Ji, Qiang; Bell, Shaun W.; Holben, Brent N.; Ellsworth, Welton J.; Roush, Ted L.; Zhang, Wu; Huang, J.; hide

    2012-01-01

    Tiny suspensions of solid particles or liquid droplets, called aerosols, hover in earth's atmosphere and can be found over just about anywhere including oceans, deserts, vegetated areas, and other global regions. Aerosols come in a variety of sizes, shapes, and compositions which depend on such factors as their origin and how long they have been in the atmosphere (i.e., their residence time). Some of the more common types of aerosols include mineral dust and sea salt which get lifted from the desert and ocean surfaces, respectively by mechanical forces such as strong winds. Depending on their size, aerosols will either fall out gravitationally, as in the case of larger particles, or will remain resident in the atmosphere where they can undergo further change through interactions with other aerosols and cloud particles. Not only do aerosols affect air quality where they pose a health risk, they can also perturb the distribution of radiation in the earth-atmosphere system which can inevitably lead to changes in our climate. One aerosol that has been in the forefront of many recent studies, particularly those examining its radiative effects, is mineral dust. The large spatial coverage of desert source regions and the fact that dust can radiatively interact with such a large part of the electromagnetic spectrum due to its range in particle size, makes it an important aerosol to study. Dust can directly scatter and absorb solar and infrared radiation which can subsequently alter the amount of radiation that would otherwise be present in the absence of dust at any level of the atmosphere like the surface. This is known as radiative forcing. At the surface dust can block incoming solar energy, however at infrared wavelengths, dust acts to partially compensate the solar losses. Evaluating the solar radiative effect of dust aerosols is relatively straightforward due in part to the relatively large signal-to-noise ratio in the measurements. At infrared wavelengths, on the

  10. Simultaneous UV and X-ray Spectroscopy of the Seyfert 1 Galaxy NGC 5548. I. Evidence for Dust in the UV Absorbers

    NASA Astrophysics Data System (ADS)

    Kraemer, S. B.; Crenshaw, D. M.; Gabel, J. R.; Kaastra, J. S.; Steenbrugge, K.; George, I. M.; Turner, T. J.; Yaqoob, T.; Dunn, J. P.

    2002-12-01

    We present new UV spectra of the nucleus of the Seyfert 1 galaxy NGC 5548, obtained with the Space Telescope Imaging Spectrograph at high spectral resolution (λ /Δ λ = 30,000 - 46,000), simultaneously with Chandra X-ray Observatory spectra. Taking advantage of the low UV continuum and broad emission-line fluxes, we have determined that the deepest UV absorption component covers at least a portion of the inner high-ionization narrow-line region (NLR). Assuming the NLR is fully covered, we find nonunity covering factors in the cores of several components, which increase the column density measurements of N V and C IV by factors of 1.2 to 1.9; however, the revised columns have only a minor effect on the parameters derived from our photoionization models. For the first time, we have simultaneous C IV and N V columns for component 1 (at -1040 km s-1), and find that this component cannot be an X-ray warm absorber, contrary to our previous claim (based on nonsimultaneous observations of N V and C IV). We find that dust-free models of the absorbers severely overpredict the O VI columns previously obtained with the Far Ultraviolet Spectrograph, and present arguments that this is not likely due to variability. However, models that include dust (and thereby heavily deplete carbon) are successful in matching all of the observed ionic columns, and result in substantially lower ionization parameters and total column densities compared to dust-free models. Interestingly, these models yield the exact amount of dust needed to produce the observed reddening of the inner NLR, assuming a Galactic dust to gas ratio. The models produce little O VII and O VIII, indicating that none of the dusty UV absorbers is associated with a classic X-ray warm absorber.

  11. Vertical profiles of aerosol mass concentration derived by unmanned airborne in situ and remote sensing instruments during dust events

    NASA Astrophysics Data System (ADS)

    Mamali, Dimitra; Marinou, Eleni; Sciare, Jean; Pikridas, Michael; Kokkalis, Panagiotis; Kottas, Michael; Binietoglou, Ioannis; Tsekeri, Alexandra; Keleshis, Christos; Engelmann, Ronny; Baars, Holger; Ansmann, Albert; Amiridis, Vassilis; Russchenberg, Herman; Biskos, George

    2018-05-01

    In situ measurements using unmanned aerial vehicles (UAVs) and remote sensing observations can independently provide dense vertically resolved measurements of atmospheric aerosols, information which is strongly required in climate models. In both cases, inverting the recorded signals to useful information requires assumptions and constraints, and this can make the comparison of the results difficult. Here we compare, for the first time, vertical profiles of the aerosol mass concentration derived from light detection and ranging (lidar) observations and in situ measurements using an optical particle counter on board a UAV during moderate and weak Saharan dust episodes. Agreement between the two measurement methods was within experimental uncertainty for the coarse mode (i.e. particles having radii > 0.5 µm), where the properties of dust particles can be assumed with good accuracy. This result proves that the two techniques can be used interchangeably for determining the vertical profiles of aerosol concentrations, bringing them a step closer towards their systematic exploitation in climate models.

  12. New directions: Mineral dust and ozone - Heterogeneous chemistry

    NASA Astrophysics Data System (ADS)

    Ramachandran, S.

    2015-04-01

    Aerosols, the tiny solid or liquid particles suspended in air and produced from natural sources and anthropogenic activities, continue to contribute the largest uncertainty to radiative forcing (IPCC, 2013). Aerosol particles give rise to radiative forcing directly through scattering and absorption of solar and infrared radiation in the atmosphere. Aerosols also give rise to indirect radiative forcing by modifying the cloud optical properties and lifetimes. Among the aerosol species mineral dust and black carbon cause a warming (positive forcing) while sulphate and sea salt cause a cooling (negative forcing) of the Earth-atmosphere system. In tropics and sub-tropics mineral dust is a major contributor to aerosol loading and optical thickness. The global source strength of dust aerosol varies significantly on spatial and temporal scales. The source regions of dust are mainly deserts, dry lake beds, and semi-arid regions, in addition to drier regions where vegetation has been reduced or soil surfaces that are disturbed by man made activities. Anthropogenic activities mainly related to agriculture such as harvesting, ploughing, overgrazing, and cement production and transport also produce mineral dust. An estimated 2500 terragram (Tg, 1012 g) of mineral dust is emitted into the atmosphere per year, and dominates the aerosol mass over continental regions in south Asia and China accounting for ∼35% of the total aerosol mass (IPCC, 2013). In India, dust is prevalent throughout the north and western India during the year and peaks during premonsoon season.

  13. A View of Earth's Aerosol System from Space to Your Office Chair

    NASA Technical Reports Server (NTRS)

    Colarco, Peter

    2008-01-01

    Aerosols are tiny particles and droplets suspended in the air. Each day you breathe in about 10 billion of them, about a half a million per breath. They are formed in nature by volcanoes, dust storms, sea spray, and emissions from vegetation. Humans create aerosols and alter their natural sources by burning fossil fuels and modifying land cover. Fires are another important source of aerosols; some are natural, such as wildfires started by lightning strikes, while others are from human-caused burning of vegetation for cooking, heating, and land clearing. Aerosols have complex effects on Earth's climate. In general, they cool the surface by reflecting (scattering) radiation from the sun back into space. Dust and smoke absorb solar radiation and heat the atmosphere where they are concentrated. Aerosols change the properties of clouds. Indeed, it would be very difficult to form clouds in the atmosphere without aerosols to act as 'seeds' for water to condense on. In aerosol polluted environments clouds tend to have smaller droplets than clouds formed in cleaner environments; these polluted clouds appear brighter from space because they reflect more sunlight, and they may persist longer and not rain as intensely. Aerosols also affect local air quality and visibility. Data collected by NASA satellites over the past decade have provided an unprecedented view of Earth's aerosol distribution and dramatically increased our understanding of where aerosols come from and just how far they travel in the atmosphere. In this talk I will discuss observations of aerosols from space and how they inform numerical transport models attempting to simulate the global aerosol system.

  14. Surface Measurements of dust/local aerosol properties over Northern China during 2008 China-US joined dust field campaign

    NASA Astrophysics Data System (ADS)

    Wang, X.; Huang, J.

    2009-12-01

    The objective of this study is to understand the detailed characteristics and underlying mechanisms of aerosol physical and optical parameters over China Loess Plateau and its potential impacts on the regional/global climate. In order to characterize the emission, transport, and removal of atmospheric pollutants emitted from East Asia, the 2008 China-US joined field campaign are conducted from late April to May 2008 focused specifically on the Asian direct measurements of dust and pollution transport, following the plume from the Northern China which from the Taklamakan desert and Gobi desert to the Eastern Pacific and into North America. Such measurements are crucial to understanding how the dust and the pollution plume (including black carbon) are modified as their age. Three sites involved this campaign, including one permanent site (Semi-Arid Climate & Environment Observatory of Lanzhou University (SACOL)) (located in Yuzhong, 35.95N/104.1E), one SACOL's Mobile Facility (SMF) (deployed in Jintai, 37.57N/104.23E) and the U.S. Department of Energy Atmospheric Radiation Measurements(ARM) Ancillary Facility (AAF mobile laboratories, SMART-COMMIT) (deployed in Zhangye, 39.08N/100.27E). Results indicate that the dust plumes are transported from the surface to a long distance from their sources have a significant influence on the air quality in the study area. The meteorological analysis indicates that these polluted layers are not from local sources during dust plume and this large-scale transport of dust and pollutants remains a major uncertainty in quantifying the global effect of emissions from Northern China.

  15. Fingerprinting the Impacts of Aerosols on Long-Term Trends of the Indian Summer Monsoon Regional Rainfall

    NASA Technical Reports Server (NTRS)

    Laul, K. M.; Kim, K. M.

    2010-01-01

    In this paper, we present corroborative observational evidences from satellites, in-situ observations, and re-analysis data showing possible impacts of absorbing aerosols (black carbon and dust) on subseasonal and regional summer monsoon rainfall over India. We find that increased absorbing aerosols in the Indo-Gangetic Plain in recent decades may have lead to long-term warming of the upper troposphere over northern India and the Tibetan Plateau, enhanced rainfall in northern India and the Himalayas foothill regions in the early part (may-June) of the monsoon season, followed by diminished rainfall over central and southern India in the latter part (July-August) of the monsoon season. These signals which are consistent with current theories of atmospheric heating and solar dimming by aerosol and induced cloudiness in modulating the Indian monsoon, would have been masked by conventional method of using al-India rainfall averaged over the entire monsoon season.

  16. Electron Microscopy Characterization of Aerosols Collected at Mauna Loa Observatory During Asian Dust Storm Event

    EPA Science Inventory

    Atmospheric aerosol particles have a significant influence on global climate due to their ability to absorb and scatter incoming solar radiation. Size, composition, and morphology affect a particle’s radiative properties and these can be characterized by electron microscopy. Lo...

  17. Global and Seasonal Aerosol Optical Depths Derived From Ultraviolet Observations by Satellites (TOMS)

    NASA Technical Reports Server (NTRS)

    Herman, J. R.; Torres, O.

    1999-01-01

    It has been shown that absorbing aerosols (dust, smoke, volcanic ash) can be detected in the ultraviolet wavelengths (331 nm to 380 nm) from satellite observations (TOMS, Total Ozone Mapping Spectrometer) over both land and water. The theoretical basis for these observations and their conversions to optical depths is discussed in terms of an aerosol index AI or N-value residue (assigned positive for absorbing aerosols). The theoretical considerations show that negative values of the AI frequently represent the presence of non-absorbing aerosols (NA) in the troposphere (mostly pollution in the form of sulfates, hydrocarbons, etc., and some natural sulfate aerosols) with particle sizes near 0.1 to 0.2 microns or less. The detection of small-particle non-absorbing aerosols from the measured backscattered radiances is based on the observed wavelength dependence from Mie scattering after the background Rayleigh scattering is subtracted. The Mie scattering from larger particles, 1 micron or more (e.g., cloud water droplets) has too small a wavelength dependence to be detected by this method. In regions that are mostly cloud free, aerosols of all sizes can be seen in the single channel 380 nm or 360 nm radiance data. The most prominent Al feature observed is the strong asymmetry in aerosol amount between the Northern and Southern Hemispheres, with the large majority of NA occurring above 20degN latitude. The maximum values of non-absorbing aerosols are observed over the eastern U.S. and most of western Europe corresponding to the areas of highest industrial pollution. Annual cycles in the amount of NA are observed over Europe and North America with maxima occurring in the summer corresponding to times of minimum wind transport. Similarly, the maxima in the winter over the Atlantic Ocean occurs because of wind borne transport from the land. Most regions of the world have the maximum amount of non-absorbing aerosol in the December to January period except for the eastern

  18. Atmospheric Processing and Iron Mobilization of Ilmenite: Iron-Containing Ternary Oxide in Mineral Dust Aerosol.

    PubMed

    Hettiarachchi, Eshani; Hurab, Omar; Rubasinghege, Gayan

    2018-02-08

    Over the last several decades, iron has been identified as a limiting nutrient in about half of the world's oceans. Its most significant source is identified as deposited iron-containing mineral dust that has been processed during atmospheric transportation. The current work focuses on chemical and photochemical processing of iron-containing mineral dust particles in the presence of nitric acid, and an organic pollutant dimethyl sulfide under atmospherically relevant conditions. More importantly, ilmenite (FeTiO 3 ) is evaluated as a proxy for the iron-containing mineral dust. The presence of titanium in its lattice structure provides higher complexity to mimic mineral dust, yet it is simple enough to study reaction pathways and mechanisms. Here, spectroscopic methods are combined with dissolution measurements to investigate atmospheric processing of iron in mineral dust, with specific focus on particle mineralogy, particle size, and their environmental conditions (i.e., pH and solar flux). Our results indicate that the presence of titanium elemental composition enhances iron dissolution from mineral dust, at least by 2-fold comparison with its nontitanium-containing counterparts. The extent of iron dissolution and speciation is further influenced by the above factors. Thus, our work highlights these important, yet unconsidered, factors in the atmospheric processing of iron-containing mineral dust aerosol.

  19. Satellite and Ground-based Radiometers Reveal Much Lower Dust Absorption of Sunlight than Used in Climate Models

    NASA Technical Reports Server (NTRS)

    Kaufman, Y. J.; Tanre, D.; Dubovik, O.; Karnieli, A.; Remer, L. A.; Einaudi, Franco (Technical Monitor)

    2000-01-01

    The ability of dust to absorb solar radiation and heat the atmosphere is one of the main uncertainties in climate modeling and the prediction of climate change. Dust absorption is not well known due to limitations of in situ measurements. New techniques to measure dust absorption are needed in order to assess the impact of dust on climate. Here we report two new independent remote sensing techniques that provide sensitive measurements of dust absorption. Both are based on remote sensing. One uses satellite spectral measurements, the second uses ground based sky measurements from the AERONET network. Both techniques demonstrate that Saharan dust absorption of solar radiation is several times smaller than the current international standards. Dust cooling of the earth system in the solar spectrum is therefore significantly stronger than recent calculations indicate. We shall also address the issue of the effects of dust non-sphericity on the aerosol optical properties.

  20. Photocatalytic Oxidation of Isoprene on Hydrated Atmospheric Mineral Dusts

    NASA Astrophysics Data System (ADS)

    Hoffmann, M. R.; Kameel, F. R.; Colussi, A. J.

    2011-12-01

    Mineral dust aerosols, an important fraction in the tropospheric aerosol budget, contain transition metal-based semiconductor particles that absorb light and may support diverse chemical transformations. Dust aerosol is primary, mostly originates from deserts, but includes fly ash emitted by power plants, and can be carried over long distances. We propose that such semiconductor particles may produce secondary organic aerosol (SOA) via surface-activated photochemical processes in aqueous media. Isoprene, the most abundant anthropogenic VOC is deemed to be incorporated into SOA by various mechanisms that remain to be fully characterized. We suggest that condensed-phase chemistry, in addition to gas-phase transformations, plays an important role in SOA formation. Isoprene is only slightly soluble in water, but it would react at diffusionally-controlled rates with photochemically generated OH-radicals in aqueous phase to produce more complex, polar compounds via oxidation and polymerization processes. We have found that the similar products are formed in the photolysis of aqueous hydrogen peroxide solutions or titanium dioxide suspensions in the presence of dissolved isoprene, as revealed by HPLC analysis with online high-resolution positive ion electrospray ionization mass spectrometric detection, and 1H and 13C nuclear magnetic resonance spectrometry. In contrast, hematite suspensions display negligible photocatalytic activity toward isoprene oxidation. These results suggest that atmospheric heterogeneous semiconductor photocatalysis of isoprene may play a significant role in global secondary organic aerosol formation under overly dusty conditions. Full product characterization is underway that aims at identifying species that may have adverse health/respiratory effects.

  1. Quantifying the Aerosol Semi-Direct Effect in the NASA GEOS-5 AGCM

    NASA Technical Reports Server (NTRS)

    Randles, Cynthia A.; Colarco, Peter R.; daSilva, Arlindo

    2011-01-01

    Aerosols such as black carbon, dust, and some organic carbon species both scatter and absorb incoming solar radiation. This direct aerosol radiative forcing (DARF) redistributes solar energy both by cooling the surface and warming the atmosphere. As a result, these aerosols affect atmospheric stability and cloud cover (the semi-direct effect, or SDE). Furthermore, in regions with persistent high loadings of absorbing aerosols (e.g. Asia), regional circulation patterns may be altered, potentially resulting in changes in precipitation patterns. Here we investigate aerosol-climate coupling using the NASA Goddard Earth Observing System model version 5 (GEOS-5) atmospheric general circulation model (AGCM), in which we have implemented an online version of the Goddard Chemistry, Aerosol, Radiation and Transport (GOCART) model. GOCART includes representations of the sources, sinks, and chemical transformation of externally mixed dust, sea salt, sulfate, and carbonaceous aerosols. We examine a series of free-running ensemble climate simulations of the present-day period (2000-2009) forced by observed sea surface temperatures to determine the impact of aerosols on the model climate. The SDE and response of each simulation is determined by differencing with respect to the control simulation (no aerosol forcing). In a free-running model, any estimate of the SDE includes changes in clouds due both to atmospheric heating from aerosols and changes in circulation. To try and quantify the SDE without these circulation changes we then examine the DARF and SDE in GEOS-5 with prescribed meteorological analyses introduced by the MERRA analysis. By doing so, we are able to examine changes in model clouds that occur on shorter scales (six hours). In the GEOS-5 data assimilation system (DAS), the analysis is defined as the best estimate of the atmospheric state at any given time, and it is determined by optimally combining a first-guess short-term GCM forecast with all available

  2. Interrelationships Between Aerosol Characteristics and Light Scattering During Late-winter in a Eastern Mediterranean Arid Environment

    NASA Technical Reports Server (NTRS)

    Ichoku, C.; Andreae, M. O.; Meixner, F. X.; Schebeske, G.; Formenti, P.; Maenhaut, W.; Cafmeyer, J.; Ptasinski, J.; Karnieli, A.; Orlovsky, L.

    1999-01-01

    An intensive field campaign involving measurement of various aerosol physical, chemical, and radiative properties was conducted at Sde Boker in the Negev Desert of Israel, from 18 February to 15 March 1997. Nephelometer measurements gave average background scattering coefficient values of about 25 M/m at 550 nm wavelength, but strong dust events caused the value of this parameter to rise up to about 800 M/m Backscattering fractions did not depend on aerosol loading, and generally fell in the range of 0.1 to 0.25, comparable to values reported for marine and Arctic environments. Chemical analysis of the aerosol revealed that, in the coarse size range (2 - 10 micrometer equivalent aerodynamic diameter (EAD)), calcium (Ca) was by far the most abundant element followed by silicon (Si), both of which are indicators for mineral dust. In the fine size fraction (< 2 micrometers EAD), sulfur (S) generally was the dominant element, except during high dust episodes when Ca and Si were again the most abundant. Furthermore, fine black carbon (BC) correlates with S, suggesting that they may have originated from the same sources or source regions. An indication of the short-term effect of aerosol loading on radiative forcing was provided by measurements of global and diffuse solar radiation, which showed that during high turbidity periods (strong dust events) almost all of the solar radiation reaching the area is scattered or absorbed.

  3. Interrelationships between aerosol characteristics and light scattering during late winter in an Eastern Mediterranean arid environment

    NASA Astrophysics Data System (ADS)

    Ichoku, Charles; Andreae, Meinrat O.; Andreae, Tracey W.; Meixner, Franz X.; Schebeske, Guenther; Formenti, Paola; Maenhaut, Willy; Cafmeyer, Jan; Ptasinski, Jacek; Karnieli, Arnon; Orlovsky, Leah

    1999-10-01

    An intensive field campaign involving measurement of various aerosol physical, chemical, and radiative properties was conducted at Sde Boker (also written as Sede Boqer) in the Negev Desert of Israel, from 18 February to 15 March 1997. Nephelometer measurements gave average background scattering coefficient values of about 25 Mm-1 at 550 nm wavelength, but strong dust events caused the value of this parameter to rise up to about 800 Mm-1. Backscattering fractions did not depend on aerosol loading and generally fell in the range of 0.1 to 0.25, comparable to values reported for marine and Arctic environments. Chemical analysis of the aerosol revealed that in the coarse size range (2-10 μm equivalent aerodynamic diameter (EAD)), calcium (Ca) was by far the most abundant element followed by silicon (Si), both of which are indicators for mineral dust. In the fine size fraction (<2 μm EAD), sulfur (S) generally was the dominant element, except during high dust episodes when Ca and Si were again the most abundant. Furthermore, fine black carbon (BC) correlates with S, suggesting that they may have originated from the same sources or source regions. An indication of the short-term effect of aerosol loading on radiative forcing was provided by measurements of global and diffuse solar radiation, which showed that during high-turbidity periods (strong dust events), almost all of the solar radiation reaching the area is scattered or absorbed.

  4. Optical-microphysical properties of Saharan dust aerosols and composition relationship using a multi-wavelength Raman lidar, in situ sensors and modelling: a case study analysis

    NASA Astrophysics Data System (ADS)

    Papayannis, A.; Mamouri, R. E.; Amiridis, V.; Remoundaki, E.; Tsaknakis, G.; Kokkalis, P.; Veselovskii, I.; Kolgotin, A.; Nenes, A.; Fountoukis, C.

    2012-05-01

    A strong Saharan dust event that occurred over the city of Athens, Greece (37.9° N, 23.6° E) between 27 March and 3 April 2009 was followed by a synergy of three instruments: a 6-wavelength Raman lidar, a CIMEL sun-sky radiometer and the MODIS sensor. The BSC-DREAM model was used to forecast the dust event and to simulate the vertical profiles of the aerosol concentration. Due to mixture of dust particles with low clouds during most of the reported period, the dust event could be followed by the lidar only during the cloud-free day of 2 April 2009. The lidar data obtained were used to retrieve the vertical profile of the optical (extinction and backscatter coefficients) properties of aerosols in the troposphere. The aerosol optical depth (AOD) values derived from the CIMEL ranged from 0.33-0.91 (355 nm) to 0.18-0.60 (532 nm), while the lidar ratio (LR) values retrieved from the Raman lidar ranged within 75-100 sr (355 nm) and 45-75 sr (532 nm). Inside a selected dust layer region, between 1.8 and 3.5 km height, mean LR values were 83 ± 7 and 54 ± 7 sr, at 355 and 532 nm, respectively, while the Ångström-backscatter-related (ABR355/532) and Ångström-extinction-related (AER355/532) were found larger than 1 (1.17 ± 0.08 and 1.11 ± 0.02, respectively), indicating mixing of dust with other particles. Additionally, a retrieval technique representing dust as a mixture of spheres and spheroids was used to derive the mean aerosol microphysical properties (mean and effective radius, number, surface and volume density, and mean refractive index) inside the selected atmospheric layers. Thus, the mean value of the retrieved refractive index was found to be 1.49( ± 0.10) + 0.007( ± 0.007)i, and that of the effective radiuses was 0.30 ± 0.18 μm. The final data set of the aerosol optical and microphysical properties along with the water vapor profiles obtained by Raman lidar were incorporated into the ISORROPIA II model to provide a possible aerosol composition

  5. Influence of crustal dust and sea spray supermicron particle concentrations and acidity on inorganic NO 3 − aerosol during the 2013 Southern Oxidant and Aerosol Study

    DOE PAGES

    Allen, H. M.; Draper, D. C.; Ayres, B. R.; ...

    2015-09-25

    Inorganic aerosol composition was measured in the southeastern United States, a region that exhibits high aerosol mass loading during the summer, as part of the 2013 Southern Oxidant and Aerosol Study (SOAS) campaign. Measurements using a Monitor for AeRosols and GAses (MARGA) revealed two periods of high aerosol nitrate (NO 3 −) concentrations during the campaign. These periods of high nitrate were correlated with increased concentrations of supermicron crustal and sea spray aerosol species, particularly Na + and Ca 2+, and with a shift towards aerosol with larger (1 to 2.5 μm) diameters. We suggest this nitrate aerosol forms bymore » multiphase reactions of HNO 3 and particles, reactions that are facilitated by transport of crustal dust and sea spray aerosol from a source within the United States. The observed high aerosol acidity prevents the formation of NH 4NO 3, the inorganic nitrogen species often dominant in fine-mode aerosol at higher pH. In addition, calculation of the rate of the heterogeneous uptake of HNO 3 on mineral aerosol supports the conclusion that aerosol NO 3 − is produced primarily by this process, and is likely limited by the availability of mineral cation-containing aerosol surface area. Modeling of NO 3 − and HNO 3 by thermodynamic equilibrium models (ISORROPIA II and E-AIM) reveals the importance of including mineral cations in the southeastern United States to accurately balance ion species and predict gas–aerosol phase partitioning.« less

  6. The fertilizing role of African dust in the Amazon rainforest: A first multiyear assessment based on data from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations

    NASA Astrophysics Data System (ADS)

    Yu, Hongbin; Chin, Mian; Yuan, Tianle; Bian, Huisheng; Remer, Lorraine A.; Prospero, Joseph M.; Omar, Ali; Winker, David; Yang, Yuekui; Zhang, Yan; Zhang, Zhibo; Zhao, Chun

    2015-03-01

    The productivity of the Amazon rainforest is constrained by the availability of nutrients, in particular phosphorus (P). Deposition of long-range transported African dust is recognized as a potentially important but poorly quantified source of phosphorus. This study provides a first multiyear satellite-based estimate of dust deposition into the Amazon Basin using three-dimensional (3-D) aerosol measurements over 2007-2013 from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The 7 year average of dust deposition into the Amazon Basin is estimated to be 28 (8-48) Tg a-1 or 29 (8-50) kg ha-1 a-1. The dust deposition shows significant interannual variation that is negatively correlated with the prior-year rainfall in the Sahel. The CALIOP-based multiyear mean estimate of dust deposition matches better with estimates from in situ measurements and model simulations than a previous satellite-based estimate does. The closer agreement benefits from a more realistic geographic definition of the Amazon Basin and inclusion of meridional dust transport calculation in addition to the 3-D nature of CALIOP aerosol measurements. The imported dust could provide about 0.022 (0.006-0.037) Tg P of phosphorus per year, equivalent to 23 (7-39) g P ha-1 a-1 to fertilize the Amazon rainforest. This out-of-basin phosphorus input is comparable to the hydrological loss of phosphorus from the basin, suggesting an important role of African dust in preventing phosphorus depletion on timescales of decades to centuries.

  7. Interstellar silicate dust in the z = 0.685 absorber toward TXS 0218+357

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Aller, Monique C.; Kulkarni, Varsha P.; Liger, Nicholas

    2014-04-10

    We report the detection of interstellar silicate dust in the z {sub abs} = 0.685 absorber along the sightline toward the gravitationally lensed blazar TXS 0218+357. Using Spitzer Space Telescope Infrared Spectrograph data, we detect the 10 μm silicate absorption feature with a detection significance of 10.7σ. We fit laboratory-derived silicate dust profile templates obtained from the literature to the observed 10 μm absorption feature and find that the best single-mineral fit is obtained using an amorphous olivine template with a measured peak optical depth of τ{sub 10} = 0.49 ± 0.02, which rises to τ{sub 10} ∼ 0.67 ±more » 0.04 if the covering factor is taken into account. We also detected the 18 μm silicate absorption feature in our data with a >3σ significance. Due to the proximity of the 18 μm absorption feature to the edge of our covered spectral range, and associated uncertainty about the shape of the quasar continuum normalization near 18 μm, we do not independently fit this feature. We find, however, that the shape and depth of the 18 μm silicate absorption are well matched to the amorphous olivine template prediction, given the optical depth inferred for the 10 μm feature. The measured 10 μm peak optical depth in this absorber is significantly higher than those found in previously studied quasar absorption systems. However, the reddening, 21 cm absorption, and velocity spread of Mg II are not outliers relative to other studied absorption systems. This high optical depth may be evidence for variations in dust grain properties in the interstellar medium between this and the previously studied high redshift galaxies.« less

  8. Lessons learned and way forward from 6 years of Aerosol_cci

    NASA Astrophysics Data System (ADS)

    Popp, Thomas; de Leeuw, Gerrit; Pinnock, Simon

    2017-04-01

    Within the ESA Climate Change Initiative (CCI) Aerosol_cci (2010 - 2017) conducts intensive work to improve and qualify algorithms for the retrieval of aerosol information from European sensors. Meanwhile, several validated (multi-) decadal time series of different aerosol parameters from complementary sensors are available: Aerosol Optical Depth (AOD), stratospheric extinction profiles, a qualitative Absorbing Aerosol Index (AAI), fine mode AOD, mineral dust AOD; absorption information and aerosol layer height are in an evaluation phase and the multi-pixel GRASP algorithm for the POLDER instrument is used for selected regions. Validation (vs. AERONET, MAN) and inter-comparison to other satellite datasets (MODIS, MISR, SeaWIFS) proved the high quality of the available datasets comparable to other satellite retrievals and revealed needs for algorithm improvement (for example for higher AOD values) which were taken into account in an iterative evolution cycle. The datasets contain pixel level uncertainty estimates which were also validated and improved in the reprocessing. The use of an ensemble method was tested, where several algorithms are applied to the same sensor. The presentation will summarize and discuss the lessons learned from the 6 years of intensive collaboration and highlight major achievements (significantly improved AOD quality, fine mode AOD, dust AOD, pixel level uncertainties, ensemble approach); also limitations and remaining deficits shall be discussed. An outlook will discuss the way forward for the continuous algorithm improvement and re-processing together with opportunities for time series extension with successor instruments of the Sentinel family and the complementarity of the different satellite aerosol products.

  9. Spatiotemporal variability and contribution of different aerosol types to the Aerosol Optical Depth over the Eastern Mediterranean.

    PubMed

    Georgoulias, Aristeidis K; Alexandri, Georgia; Kourtidis, Konstantinos A; Lelieveld, Jos; Zanis, Prodromos; Pöschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2016-01-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the Aerosol Optical Depth (AOD) over the Eastern Mediterranean as derived from MODIS Terra (3/2000-12/2012) and Aqua (7/2002-12/2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sunphotometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium sized cities, industrial zones, and power plant complexes, seasonal variabilities, and decadal averages. The average AOD at 550 nm (AOD 550 ) for the entire region is ~ 0.22 ± 0.19 with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in Central and Eastern Europe, and transport of dust from the Sahara Desert and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD 550 . The spatial and temporal variability of anthropogenic, dust and fine mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD 550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine mode natural aerosols account for ~ 51 %, ~ 34 % and ~ 15 % of the total AOD 550 over land, while, anthropogenic aerosols, dust and marine aerosols account ~ 40 %, ~ 34 % and ~ 26 % of the total AOD 550 over the sea, based on MODIS Terra and Aqua observations.

  10. Analysis of MAIAC Dust Aerosol Retrievals from MODIS Over North Africa

    NASA Technical Reports Server (NTRS)

    Lyapustin, A.; Wang, Y.; Hsu, C.; Torres, O.; Leptoukh, G.; Kalashnikova, O.; Korkin, S.

    2011-01-01

    An initial comparison of aerosol optical thickness over North Africa for year 2007 was performed between the Deep Blue and Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithms complimented with MISR and OMI data. The new MAIAC algorithm has a better sensitivity to the small dust storms than the DB algorithm, but it also has biases in the brightest desert regions indicating the need for improvement. The quarterly averaged AOT values in the Bodele depression and western downwind transport region show a good agreement among MAIAC, MISR and OMI data, while the DB algorithm shows a somewhat different seasonality.

  11. A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-Cloud Aerosols Using CALIOP and MODIS Data

    NASA Technical Reports Server (NTRS)

    Zhang, Z.; Meyer, K.; Platnick, S.; Oreopoulos, L.; Lee, D.; Yu, H.

    2014-01-01

    This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.

  12. Direct Radiative Effect of Intense Dust Outbreaks in the Mediterranean

    NASA Astrophysics Data System (ADS)

    Gkikas, A.; Obiso, V.; Basart, S.; Jorba, O.; Pérez García-Pando, C.; Hatzianastassiou, N.; Gassó, S.; Baldasano, J. M.

    2015-12-01

    The broader Mediterranean basin is affected by intense desert dust outbreaks in spring. In the present study, we make use of satellite observations and modelling to investigate dust radiative impacts during three consecutive dust outbreaks occurred over the Mediterranean in the period 9/4-15/4/2008. The direct radiative effect (DRE) is estimated by using two simulations run with the NMMB/BSC-Dust model, where the interaction between dust aerosols and radiation is activated and deactivated, respectively. The simulation domain covers the North Africa, the Middle East and Europe at 0.25ºx0.25° and 40σ-layers. The first outbreak took place over the central and eastern Mediterranean on the 9th reaching aerosol optical depths (AODs) close to 1. The second one, with AODs up to 2, lasted from 10th to 14th affecting mainly the central Mediterranean. The third one, with AODs up to 5, affected the Iberian Peninsula on the 15th. DREs are computed for the outgoing radiation at the top of the atmosphere (TOA), the absorbed radiation into the atmosphere (ATMAB), for the downwelling (SURF) and the absorbed (NETSURF) radiation at surface, for the shortwave (SW), longwave (LW) and NET (SW+LW) radiation. According to our results, it is evident that DREs' spatial patterns are driven by those of AOD. Negative (cooling) instantaneous DRETOA, DRESURF and DRENETSURF values up to -500W/m2, -700W/m2 and -600W/m2, respectively, and positive (warming) instantaneous DREATMAB up to 340W/m2 are found for the SW spectrum, during daytime. Opposite but less pronounced effects are encountered for the LW radiation and during nightime. Due to these perturbations on the radiation field, the surface temperature is reduced locally by up to 8°C during daytime and increased by up to 4°C during nightime. It is found that the regional average NET DREs can be as large as -12W/m2, -45W/m2, -30W/m2 and 27W/m2 for TOA, SURF, NETSURF and ATMAB, respectively. Impacts on atmospheric stability and dust

  13. Airborne lidar measurements to investigate the impact of long-range transported dust on shallow marine trade wind convection

    NASA Astrophysics Data System (ADS)

    Gross, S.; Gutleben, M.; Wirth, M.; Ewald, F.

    2017-12-01

    Aerosols and clouds are still main contributors to uncertainties in estimates and interpretation of the Earth's changing energy budget. Their interaction with the Earth's radiation budged has a direct component by scattering and absorbing solar and terrestrial radiation, and an indirect component, e.g. as aerosols modify the properties and thus the life-time of clouds or by changing the atmosphere's stability. Up to know now sufficient understanding in aerosol-cloud interaction and climate feedback is achieved. Thus studies with respect to clouds, aerosols, their interaction and influence on the radiation budged are highly demanded. In August 2016 the NARVAL-II (Next-generation airborne remote sensing for validation studies) mission took place. Measurements with a combined active (high spectral resolution and water vapor differential absorption lidar and cloud radar) and passive remote sensing (microwave radiometer, hyper spectral imager, radiation measurements) payload were performed with the German high altitude and long-range research aircraft HALO over the subtropical North-Atlantic Ocean to study shallow marine convection during the wet and dusty season. With this, NARVAL-II is follow-up of the NARVAL-I mission which took place during the dry and dust free season in December 2013. During NARVAL-II the measurement flights were designed the way to sample dust influenced areas as well as dust free areas in the trades. One main objective was to investigate the optical and macro physical properties of the dust layer, differences in cloud occurrence in dusty and non-dusty areas, and to study the influence of aerosols on the cloud properties and formation. This allows comparisons of cloud and aerosol distribution as well as their environment between the dry and the wet season, and of cloud properties and distribution with and without the influence of long-range transported dust across the Atlantic Ocean. In our presentation we will give an overview of the NARVAL

  14. Aerosol loading impact on Asian monsoon precipitation patterns

    NASA Astrophysics Data System (ADS)

    Biondi, Riccardo; Cagnazzo, Chiara; Costabile, Francesca; Cairo, Francesco

    2017-04-01

    Solar light absorption by aerosols such as black carbon and dust assume a key role in driving the precipitation patterns in the Indian subcontinent. The aerosols stack up against the foothills of the Himalayas in the pre-monsoon season and several studies have already demonstrated that this can cause precipitation anomalies during summer. Despite its great significance in climate change studies, the link between absorbing aerosols loading and precipitation patterns remains highly uncertain. The main challenge for this kind of studies is to find consistent and reliable datasets. Several aerosol time series are available from satellite and ground based instruments and some precipitation datasets from satellite sensors, but they all have different time/spatial resolution and they use different assumptions for estimating the parameter of interest. We have used the aerosol estimations from the Ozone Monitoring Instrument (OMI), the Along-Track Scanning Radiometer (AATSR) and the MODerate resolution Imaging Spectroradiometer (MODIS) and validated them against the Aerosol Robotic Network (AERONET) measurements in the Indian area. The precipitation has been analyzed by using the Tropical Rainfall Measuring Mission (TRMM) estimations and the Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2). From our results it is evident the discrepancy between the aerosol loading on the area of interest from the OMI, AATSR, and MODIS, but even between 3 different algorithms applied to the MODIS data. This uncertainty does not allow to clearly distinguishing high aerosol loading years from low aerosol loading years except in a couple of cases where all the estimations agree. Similar issues are also present in the precipitation estimations from TRMM and MERRA-2. However, all the aerosol datasets agree in defining couples of consecutive years with a large gradient of aerosol loading. Based on this assumption we have compared the precipitation anomalies and

  15. Evolution of trace elements in the planetary boundary layer in southern China: Effects of dust storms and aerosol-cloud interactions

    NASA Astrophysics Data System (ADS)

    Li, Tao; Wang, Yan; Zhou, Jie; Wang, Tao; Ding, Aijun; Nie, Wei; Xue, Likun; Wang, Xinfeng; Wang, Wenxing

    2017-03-01

    Aerosols and cloud water were analyzed at a mountaintop in the planetary boundary layer in southern China during March-May 2009, when two Asian dust storms occurred, to investigate the effects of aerosol-cloud interactions (ACIs) on chemical evolution of atmospheric trace elements. Fe, Al, and Zn predominated in both coarse and fine aerosols, followed by high concentrations of toxic Pb, As, and Cd. Most of these aerosol trace elements, which were affected by dust storms, exhibited various increases in concentrations but consistent decreases in solubility. Zn, Fe, Al, and Pb were the most abundant trace elements in cloud water. The trace element concentrations exhibited logarithmic inverse relationships with the cloud liquid water content and were found highly pH dependent with minimum concentrations at the threshold of pH 5.0. The calculation of Visual MINTEQ model showed that 80.7-96.3% of Fe(II), Zn(II), Pb(II), and Cu(II) existed in divalent free ions, while 71.7% of Fe(III) and 71.5% of Al(III) were complexed by oxalate and fluoride, respectively. ACIs could markedly change the speciation distributions of trace elements in cloud water by pH modification. The in-cloud scavenging of aerosol trace elements likely reached a peak after the first 2-3 h of cloud processing, with scavenging ratios between 0.12 for Cr and 0.57 for Pb. The increases of the trace element solubility (4-33%) were determined in both in-cloud aerosols and postcloud aerosols. These results indicated the significant importance of aerosol-cloud interactions to the evolution of trace elements during the first several cloud condensation/evaporation cycles.

  16. Estimating the Direct Radiative Effect of Absorbing Aerosols Overlying Marine Boundary Layer Clouds in the Southeast Atlantic Using MODIS and CALIOP

    NASA Technical Reports Server (NTRS)

    Meyer, Kerry; Platnick, Steven; Oreopoulos, Lazaros; Lee, Dongmin

    2013-01-01

    Absorbing aerosols such as smoke strongly absorb solar radiation, particularly at ultraviolet and visible/near-infrared (VIS/NIR) wavelengths, and their presence above clouds can have considerable implications. It has been previously shown that they have a positive (i.e., warming) direct aerosol radiative effect (DARE) when overlying bright clouds. Additionally, they can cause biased passive instrument satellite retrievals in techniques that rely on VIS/NIR wavelengths for inferring the cloud optical thickness (COT) and effective radius (re) of underlying clouds, which can in turn yield biased above-cloud DARE estimates. Here we investigate Moderate Resolution Imaging Spectroradiometer (MODIS) cloud optical property retrieval biases due to overlying absorbing aerosols observed by Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and examine the impact of these biases on above-cloud DARE estimates. The investigation focuses on a region in the southeast Atlantic Ocean during August and September (2006-2011), where smoke from biomass burning in southern Africa overlies persistent marine boundary layer stratocumulus clouds. Adjusting for above-cloud aerosol attenuation yields increases in the regional mean liquid COT (averaged over all ocean-only liquid clouds) by roughly 6%; mean re increases by roughly 2.6%, almost exclusively due to the COT adjustment in the non-orthogonal retrieval space. It is found that these two biases lead to an underestimate of DARE. For liquid cloud Aqua MODIS pixels with CALIOP-observed above-cloud smoke, the regional mean above-cloud radiative forcing efficiency (DARE per unit aerosol optical depth (AOD)) at time of observation (near local noon for Aqua overpass) increases from 50.9Wm(sup-2)AOD(sup-1) to 65.1Wm(sup-2)AOD(sup -1) when using bias-adjusted instead of nonadjusted MODIS cloud retrievals.

  17. Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

    NASA Technical Reports Server (NTRS)

    Quinn, P. K.; Coffman, D. J.; Bates, T. S.; Welton, E. J.; Covert, D. S.; Miller, T. L.; Johnson, J. E.; Maria, S.; Russell, L.; Arimoto, R.

    2004-01-01

    During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic

  18. Radiative effects of light-absorbing particles deposited in snow over Himalayas using WRF-Chem simulations

    NASA Astrophysics Data System (ADS)

    Sarangi, C.; Qian, Y.; Painter, T. H.; Liu, Y.; Lin, G.; Wang, H.

    2017-12-01

    Radiative forcing induced by light-absorbing particles (LAP) deposited on snow is an important surface forcing. It has been debated that an aerosol-induced increase in atmospheric and surface warming over Tibetan Plateau (TP) prior to the South Asian summer monsoon can have a significant effect on the regional thermodynamics and South Asian monsoon circulation. However, knowledge about the radiative effects due to deposition of LAP in snow over TP is limited. In this study we have used a high-resolution WRF-Chem (coupled with online chemistry and snow-LAP-radiation model) simulations during 2013-2014 to estimate the spatio-temporal variation in LAP deposition on snow, specifically black carbon (BC) and dust particles, in Himalayas. Simulated distributions in meteorology, aerosol concentrations, snow albedo, snow grain size and snow depth are evaluated against satellite and in-situ measurements. The spatio-temporal change in snow albedo and snow grain size with variation in LAP deposition is investigated and the resulting shortwave LAP radiative forcing at surface is calculated. The LAP-radiative forcing due to aerosol deposition, both BC and dust, is higher in magnitude over Himalayan slopes (terrain height below 4 km) compared to that over TP (terrain height above 4 km). We found that the shortwave aerosol radiative forcing efficiency at surface due to increase in deposited mass of BC particles in snow layer ( 25 (W/m2)/ (mg/m2)) is manifold higher than the efficiency of dust particles ( 0.1 (W/m2)/ (mg/m2)) over TP. However, the radiative forcing of dust deposited in snow is similar in magnitude (maximum 20-30 W/m2) to that of BC deposited in snow over TP. This is mainly because the amount of dust deposited in snow over TP can be about 100 times greater than the amount of BC deposited in snow during polluted conditions. The impact of LAP on surface energy balance, snow melting and atmospheric thermodynamics is also examined.

  19. Advantages of measuring the Q Stokes parameter in addition to the total radiance I in the detection of absorbing aerosols

    NASA Astrophysics Data System (ADS)

    Stamnes, Snorre; Fan, Yongzhen; Chen, Nan; Li, Wei; Tanikawa, Tomonori; Lin, Zhenyi; Liu, Xu; Burton, Sharon; Omar, Ali; Stamnes, Jakob J.; Cairns, Brian; Stamnes, Knut

    2018-05-01

    A simple but novel study was conducted to investigate whether an imager-type spectroradiometer instrument like MODIS, currently flying on board the Aqua and Terra satellites, or MERIS, which flew on board Envisat, could detect absorbing aerosols if they could measure the Q Stokes parameter in addition to the total radiance I, that is if they could also measure the linear polarization of the light. Accurate radiative transfer calculations were used to train a fast neural network forward model, which together with a simple statistical optimal estimation scheme was used to retrieve three aerosol parameters: aerosol optical depth at 869 nm, optical depth fraction of fine mode (absorbing) aerosols at 869 nm, and aerosol vertical location. The aerosols were assumed to be bimodal, each with a lognormal size distribution, located either between 0 and 2 km or between 2 and 4 km in the Earth's atmosphere. From simulated data with 3% random Gaussian measurement noise added for each Stokes parameter, it was found that by itself the total radiance I at the nine MODIS VIS channels was generally insufficient to accurately retrieve all three aerosol parameters (˜ 15% to 37% successful), but that together with the Q Stokes component it was possible to retrieve values of aerosol optical depth at 869 nm to ± 0.03, single-scattering albedo at 869 nm to ± 0.04, and vertical location in ˜ 65% of the cases. This proof-of-concept retrieval algorithm uses neural networks to overcome the computational burdens of using vector radiative transfer to accurately simulate top-of-atmosphere (TOA) total and polarized radiances, enabling optimal estimation techniques to exploit information from multiple channels. Therefore such an algorithm could, in concept, be readily implemented for operational retrieval of aerosol and ocean products from moderate or hyperspectral spectroradiometers.

  20. Simulation of the Aerosol-Atmosphere Interaction in the Dead Sea Area with COSMO-ART

    NASA Astrophysics Data System (ADS)

    Vogel, Bernhard; Bangert, Max; Kottmeier, Christoph; Rieger, Daniel; Schad, Tobias; Vogel, Heike

    2014-05-01

    The Dead Sea is a unique environment located in the Dead Sea Rift Valley. The fault system of the Dead Sea Rift Valley marks the political borders between Israel, Jordan, and Palestine. The Dead Sea region and the ambient Eastern Mediterranean coastal zone provide a natural laboratory for studying atmospheric processes ranging from the smallest scale of cloud processes to regional weather and climate. The virtual institute DESERVE is designed as a cross-disciplinary and cooperative international project of the Helmholtz Centers KIT, GFZ, and UFZ with well-established partners in Israel, Jordan and Palestine. One main focus of one of the work packages is the role of aerosols in modifying clouds and precipitation and in developing the Dead Sea haze layer as one of the most intriguing questions. The haze influences visibility, solar radiation, and evaporation and may even affect economy and health. We applied the online coupled model system COSMO-ART, which is able to treat the feedback processes between aerosol, radiation, and cloud formation, for a case study above the Dead Sea and adjacent regions. Natural aerosol like mineral dust and sea salt as well as anthropogenic primary and secondary aerosol is taken into account. Some of the observed features like the vertical double structure of the haze layer are already covered by the simulation. We found that absorbing aerosol like mineral dust causes a temperature increase in parts of the model domain. In other areas a decrease in temperature due to cirrus clouds modified by elevated dust layers is simulated.

  1. Advancing Littoral Zone Aerosol Prediction via Holistic Studies in Regime-Dependent Flows: August 3-9, 2016 Middle East Dust Event

    NASA Astrophysics Data System (ADS)

    Solbrig, J. E.; Miller, S. D.; van den Heever, S. C.; Kreidenweis, S. M.; Oo, M. M.; Zupanski, M.; Zhang, J.; Wang, J.; Holz, R.; Albers, S. C.; Grasso, L. D.; Kliewer, A.; Bukowski, J.; Park, J.; Saleeby, S. M.; Wu, T. C.

    2017-12-01

    Coastal regions represent a complex environment for meteorological processes, their effect on aerosol distributions, and the resulting impacts of those aerosols. These regions are rife with discontinuities that make dynamical processes difficult to predict and confound optical retrieval algorithms with highly variable and poorly characterized backgrounds. Local dynamics can be complicated by interactions between maritime and continental airmasses and the presence of coastal terrain. Additionally, coastal shallow water and high-turbidity produce backgrounds with high water leaving radiance which biases results from remote sensing retrievals. Here we present the highlights of the first two years of work from a Multi-disciplinary University Research Initiative entitled Holistic Analysis of Aerosol in Littoral Environments (HAALE-MURI) with specific focus on a dust event that occurred during the period of August 3-9 2016. During this period, two large dust plumes were observed advecting across the Arabian Peninsula. The first, embedded in a dry airmass, moved across the peninsula from north-west to south-east. This plume eventually stalls as it encounters a moist airmass, likely driven by the sea breeze. Embedded in the moist airmass is a second dust plume lofted from Oman, which then advects northwards over the Persian Gulf. This case presents significant challenges for forecasting, remote sensing, and data assimilation due to a complex meteorological environment and variable coastal bright-water backgrounds. The project team, who endeavor to advance our fundamental understanding of the factors that govern aerosol distribution, optical properties, and microphysical properties in the coastal regions, have focused on this case as our first in-depth case study. We demonstrate new retrieval techniques during both day and night including retrievals over bright coastal waters, a novel approach to in-line data assimilation of aerosol properties including AOT, and the results

  2. Aerosol Models for the CALIPSO Lidar Inversion Algorithms

    NASA Technical Reports Server (NTRS)

    Omar, Ali H.; Winker, David M.; Won, Jae-Gwang

    2003-01-01

    We use measurements and models to develop aerosol models for use in the inversion algorithms for the Cloud Aerosol Lidar and Imager Pathfinder Spaceborne Observations (CALIPSO). Radiance measurements and inversions of the AErosol RObotic NETwork (AERONET1, 2) are used to group global atmospheric aerosols using optical and microphysical parameters. This study uses more than 105 records of radiance measurements, aerosol size distributions, and complex refractive indices to generate the optical properties of the aerosol at more 200 sites worldwide. These properties together with the radiance measurements are then classified using classical clustering methods to group the sites according to the type of aerosol with the greatest frequency of occurrence at each site. Six significant clusters are identified: desert dust, biomass burning, urban industrial pollution, rural background, marine, and dirty pollution. Three of these are used in the CALIPSO aerosol models to characterize desert dust, biomass burning, and polluted continental aerosols. The CALIPSO aerosol model also uses the coarse mode of desert dust and the fine mode of biomass burning to build a polluted dust model. For marine aerosol, the CALIPSO aerosol model uses measurements from the SEAS experiment 3. In addition to categorizing the aerosol types, the cluster analysis provides all the column optical and microphysical properties for each cluster.

  3. Desert Dust and Monsoon Rain

    NASA Technical Reports Server (NTRS)

    Lau, William K. M.; Kim, Kyu-Myong

    2014-01-01

    For centuries, inhabitants of the Indian subcontinent have know that heavy dust events brought on by strong winds occur frequently in the pre-monsoon season, before the onset of heavy rain. Yet scientists have never seriously considered the possibility that natural dust can affect monsoon rainfall. Up to now, most studies of the impacts of aerosols on Indian monsoon rainfall have focused on anthropogenic aerosols in the context of climate change. However, a few recent studies have show that aerosols from antropogenic and natural sources over the Indian subcontinent may affect the transition from break to active monsoon phases on short timescales of days to weeks. Writing in Nature Geoscience, Vinoj and colleagues describe how they have shown that desert dust aerosols over the Arabian Sea and West Asia can strenghten the summer monsoon over the Indial subcontinent in a matter of days.

  4. Radiative Effects of Aerosols

    NASA Technical Reports Server (NTRS)

    Valero, Francisco P. J.

    1996-01-01

    During the Atlantic Stratocumulus Transition Experiment (ASTEX) in June 1992, two descents in cloud-free regions allowed comparison of the change in aerosol optical depth as determined by an onboard total-direct-diffuse radiometer (TDDR) to the change calculated from measured size-resolved aerosol microphysics and chemistry. Both profiles included a pollution haze from Europe but the second also included the effect of a Saharan dust layer above the haze. The separate contributions of supermicrometer (coarse) and submicrometer (fine) aerosol were determined and thermal analysis of the pollution haze indicated that the fine aerosol was composed primarily of a sulfate/water mixture with a refractory soot-like core. The soot core increased the calculated extinction by about 10% in the most polluted drier layer relative to a pure sulfate aerosol but had significantly less effect at higher humidities. A 3 km descent through a boundary layer air mass dominated by pollutant aerosol with relative humidities (RH) 10-77% yielded a close agreement between the measured and calculated aerosol optical depths (550 nm) of 0.160 (+/- 0.07) and 0. 157 (+/- 0.034) respectively. During descent the aerosol mass scattering coefficient per unit sulfate mass varied from about 5 to 16 m(exp 2)/g and primarily dependent upon ambient RH. However, the total scattering coefficient per total fine mass was far less variable at about 4+/- 0.7 m(exp 2)/g. A subsequent descent through a Saharan dust layer located above the pollution aerosol layer revealed that both layers contributed similarly to aerosol optical depth. The scattering per unit mass of the coarse aged dust was estimated at 1.1 +/- 0.2 m(exp 2)/g. The large difference (50%) in measured and calculated optical depth for the dust layer exceeded measurements.

  5. Dust Modeling with GEOS-Chem: Evidence for Acidic Uptake on Dust Surfaces during INTEX-B

    NASA Technical Reports Server (NTRS)

    Fairlie, T. Duncan

    2007-01-01

    We use measurements of aerosol ion composition and size made from the DC8 aircraft during the 2006 INTEX-B airborne campaign to identify mineral dust signatures, and look for evidence for interaction of dust with acidic components. Coating of dust with sulfate or nitrate favors the role of dust particles as cloud condensation nucleii, can promote further uptake of SO2 and N2O5, can impact NOx/HNO3 partitioning, and can shift sulfate or nitrate towards larger sizes, affecting atmospheric lifetimes for both aerosol and gas components. Mineral dust had a pervasive presence on flights made during the Northern Pacific deployment of the INTEX-B mission. We use scatter plots of ion mixing ratios with Na+ and Ca(2+) to distinguish sea salt and mineral components of the aerosol distribution, respectively. Positive correlations of non-sea-salt sulfate and nitrate with calcium indicate that the dusty air stream is associated with polluted air masses. Sulfate-ammonium scatter plots indicate sulfate to be primarily in the form of (NH4)2SO4. A positive correlation between Ca(2+) and NO-, but little evidence of NH4NO3, suggests that NO3- may be associated with mineral dust surfaces. 3-d model simulations conducted with the GEOS-Chem chemical transport model indicate that transpacific transport from East Asia was principally responsible for the dust observed from the aircraft over the Pacific. We compare the aerosol component relationships in the model with those observed. Uptake of sulfate and nitrate on the dust is not yet represented in the model.

  6. Spectral Signature of Radiative Forcing by East Asian Dust-Soot Mixture

    NASA Astrophysics Data System (ADS)

    Zhu, A.; Ramanathan, V.

    2007-12-01

    The Pacific Dust Experiment (PACDEX) provides the first detailed sampling of dust-soot mixtures from the western Pacific to the eastern Pacific Ocean. The data includes down and up spectral irradiance, mixing state of dust and soot, and other aerosol properties. This study attempts to simulate the radiative forcing by dust-soot mixtures during the experimental period. The MODTRAN band model was employed to investigate the spectral signatures of solar irradiance change induced by aerosols at moderate spectral resolutions. For the short wave band (300-1100nm) used in this study, the reduction of downward irradiance at surface by aerosols greatly enhances with increasing wavelength in the UV band (300-400nm), reaches a maximum in the blue band, then gradually decreases toward the red band. In the near-IR band (700-1100nm), irradiance reduction by aerosols shows great fluctuations in the band with center wavelength at around 940nm, 820nm, 720nm, 760nm, 690nm, where the aerosol effect is overwhelmed by the water vapor and O2 absorptions. The spectral pattern of irradiance reduction varies for different aerosol species. The maximum reduction lies at around 450nm for soot, and shifting to about 490nm for East Asian mineral dust. It's worth noting that although soot aerosols reduce more irradiance than East Asian dust in the UV and blue band, the impact of dust to the irradiance exceeds that by soot at the longer wavelength band (i.e. around 550nm). The reduction of irradiance by East Asian dust (soot) in the UV band, visible band, and near-IR accounts for about 6% (10%), 56% (64%), and 38% (26%) of total irradiance reduction. As large amount of soot aerosols are involved during the long range transport of East Asian dust, the optical properties of dust aerosols are modified with different mixing state with soot, the spectral pattern of the irradiance reduction will be changed. The study of aerosol forcing at moderate spectral resolutions has the potential application for

  7. Aerosols cause intraseasonal short-term suppression of Indian monsoon rainfall.

    PubMed

    Dave, Prashant; Bhushan, Mani; Venkataraman, Chandra

    2017-12-11

    Aerosol abundance over South Asia during the summer monsoon season, includes dust and sea-salt, as well as, anthropogenic pollution particles. Using observations during 2000-2009, here we uncover repeated short-term rainfall suppression caused by coincident aerosols, acting through atmospheric stabilization, reduction in convection and increased moisture divergence, leading to the aggravation of monsoon break conditions. In high aerosol-low rainfall regions extending across India, both in deficient and normal monsoon years, enhancements in aerosols levels, estimated as aerosol optical depth and absorbing aerosol index, acted to suppress daily rainfall anomaly, several times in a season, with lags of a few days. A higher frequency of prolonged rainfall breaks, longer than seven days, occurred in these regions. Previous studies point to monsoon rainfall weakening linked to an asymmetric inter-hemispheric energy balance change attributed to aerosols, and short-term rainfall enhancement from radiative effects of aerosols. In contrast, this study uncovers intraseasonal short-term rainfall suppression, from coincident aerosol forcing over the monsoon region, leading to aggravation of monsoon break spells. Prolonged and intense breaks in the monsoon in India are associated with rainfall deficits, which have been linked to reduced food grain production in the latter half of the twentieth century.

  8. Airborne Aerosol Closure Studies During PRIDE

    NASA Technical Reports Server (NTRS)

    Redemann, Jens; Livingston, John M.; Russell, Philip B.; Schmid, Beat; Reid, Jeff

    2000-01-01

    The Puerto Rico Dust Experiment (PRIDE) was conducted during June/July of 2000 to study the properties of Saharan dust aerosols transported across the Atlantic Ocean to the Caribbean Islands. During PRIDE, the NASA Ames Research Center six-channel (380 - 1020 nm) airborne autotracking sunphotometer (AATS-6) was operated aboard a Piper Navajo airplane alongside a suite of in situ aerosol instruments. The in situ aerosol instrumentation relevant to this paper included a Forward Scattering Spectrometer Probe (FSSP-100) and a Passive Cavity Aerosol Spectrometer Probe (PCASP), covering the radius range of approx. 0.05 to 10 microns. The simultaneous and collocated measurement of multi-spectral aerosol optical depth and in situ particle size distribution data permits a variety of closure studies. For example, vertical profiles of aerosol optical depth obtained during local aircraft ascents and descents can be differentiated with respect to altitude and compared to extinction profiles calculated using the in situ particle size distribution data (and reasonable estimates of the aerosol index of refraction). Additionally, aerosol extinction (optical depth) spectra can be inverted to retrieve estimates of the particle size distributions, which can be compared directly to the in situ size distributions. In this paper we will report on such closure studies using data from a select number of vertical profiles at Cabras Island, Puerto Rico, including measurements in distinct Saharan Dust Layers. Preliminary results show good agreement to within 30% between mid-visible aerosol extinction derived from the AATS-6 optical depth profiles and extinction profiles forward calculated using 60s-average in situ particle size distributions and standard Saharan dust aerosol refractive indices published in the literature. In agreement with tendencies observed in previous studies, our initial results show an underestimate of aerosol extinction calculated based on the in situ size distributions

  9. Laboratory evaluation of the CIP 10 personal dust sampler.

    PubMed

    Gero, A; Tomb, T

    1988-06-01

    The "capteur individuel de poussiere" CIP 10 personal dust sampler--developed by the Centre d'Etudes et Recherches de Charbonnages de France (CERCHAR) research organization--is a small, quiet, lightweight unit which samples at a flow rate of 10 L/min. It is a three-stage sampler, using two stages to remove nonrespirable dust particles and one stage to collect the respirable fraction. Airflow through the sampler is induced by the third stage, which is a rotating collector cup that contains a fine grade sponge. Laboratory tests were conducted in a dust chamber using aerosols of Arizona road dust, coal dust and silica dust. Aerosol concentrations measured with the CIP 10 were compared to those measured with the coal mine dust personal sampler unit used in the United States. The results of this study showed that aerosol concentrations measured with the CIP 10 were linearly related to those obtained with the coal mine dust personal sampler. The relationship, however, was dependent on preselector configuration and aerosol characteristics. The collection medium allows some small particles (less than 3 microns) to pass through the sampler without being collected. As much as 13% (by weight) of the aerosol that penetrated through the preseparating stages was exhausted from the sampler.

  10. Absorbing and scattering aerosols over the source region of biomass burning emissions: Implications in the assessment of optical and radiative properties

    NASA Astrophysics Data System (ADS)

    Singh, Atinderpal; Srivastava, Rohit; Rastogi, Neeraj; Singh, Darshan

    2016-02-01

    The current study focuses on the assessment of model simulated optical and radiative properties of aerosols incorporating the measured chemical composition of aerosol samples collected at Patiala during October, 2011-February, 2012. Monthly average mass concentration of PM2.5, elemental carbon (EC), primary organic carbon (POC), water-soluble (WS) and insoluble (INS) aerosols ranged from 120 to 192, 6.2 to 7.2, 20 to 39, 59 to 111 and 35 to 90 μg m-3, respectively. Mass concentration of different components of aerosols was further used for the assessment of optical properties derived from Optical Properties of Aerosols and Clouds (OPAC) model simulations. Microtops based measured aerosol optical depth (AOD500) ranged from 0.47 to 0.62 showing maximum value during November and December, and minimum during February. Ångström exponent (α380-870) remained high (>0.90) throughout the study period except in February (0.74), suggesting predominance of fine mode particles over the study region. The observed ratio of scattering to absorbing aerosols was incorporated in OPAC model simulations and single scattering albedo (SSA at 500 nm) so obtained ranged between 0.80 and 0.92 with relatively low values during the period of extensive biomass burning. In the present study, SBDART based estimated values of aerosol radiative forcing (ARF) at the surface (SRF) and top of the atmosphere (TOA) ranged from -31 to -66 Wm-2 and -2 to -18 W m-2 respectively. The atmospheric ARF, ranged between + 18 and + 58 Wm-2 resulting in the atmospheric heating rate between 0.5 and 1.6 K day-1. These results signify the role of scattering and absorbing aerosols in affecting the magnitude of aerosol forcing.

  11. Predicting the Mineral Composition of Dust Aerosols. Part 2; Model Evaluation and Identification of Key Processes with Observations

    NASA Technical Reports Server (NTRS)

    Perlwitz, J. P.; Garcia-Pando, C. Perez; Miller, R. L.

    2015-01-01

    A global compilation of nearly sixty measurement studies is used to evaluate two methods of simulating the mineral composition of dust aerosols in an Earth system model. Both methods are based upon a Mean Mineralogical Table (MMT) that relates the soil mineral fractions to a global atlas of arid soil type. The Soil Mineral Fraction (SMF) method assumes that the aerosol mineral fractions match the fractions of the soil. The MMT is based upon soil measurements after wet sieving, a process that destroys aggregates of soil particles that would have been emitted from the original, undisturbed soil. The second method approximately reconstructs the emitted aggregates. This model is referred to as the Aerosol Mineral Fraction (AMF) method because the mineral fractions of the aerosols differ from those of the wet-sieved parent soil, partly due to reaggregation. The AMF method remedies some of the deficiencies of the SMF method in comparison to observations. Only the AMF method exhibits phyllosilicate mass at silt sizes, where they are abundant according to observations. In addition, the AMF quartz fraction of silt particles is in better agreement with measured values, in contrast to the overestimated SMF fraction. Measurements at distinct clay and silt particle sizes are shown to be more useful for evaluation of the models, in contrast to the sum over all particles sizes that is susceptible to compensating errors, as illustrated by the SMF experiment. Model errors suggest that allocation of the emitted silt fraction of each mineral into the corresponding transported size categories is an important remaining source of uncertainty. Evaluation of both models and the MMT is hindered by the limited number of size-resolved measurements of mineral content that sparsely sample aerosols from the major dust sources. The importance of climate processes dependent upon aerosol mineral composition shows the need for global and routine mineral measurements.

  12. A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-cloud Aerosols over Ocean Using CALIOP and MODIS Data

    NASA Technical Reports Server (NTRS)

    Zhang, Z.; Meyer, K.; Platnick, S.; Oreopoulos, L.; Lee, D.; Yu, H.

    2013-01-01

    This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4%. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.

  13. Decadal-scale trends in regional aerosol particle properties and their linkage to emission changes

    NASA Astrophysics Data System (ADS)

    Zhao, Bin; Jiang, Jonathan H.; Gu, Yu; Diner, David; Worden, John; Liou, Kuo-Nan; Su, Hui; Xing, Jia; Garay, Michael; Huang, Lei

    2017-05-01

    Understanding long-term trends in aerosol loading and properties is essential for evaluating the health and climatic effects of these airborne particulates as well as the effectiveness of pollution control policies. While many studies have used satellite data to examine the trends in aerosol optical depth (AOD), very few have investigated the trends in aerosol properties associated with particle size, morphology, and light absorption. In this study, we investigate decadal-scale (13-15 year) trends in aerosol loading and properties during 2001-2015 over three populous regions: the Eastern United States (EUS), Western Europe (WEU), and Eastern and Central China (ECC). We use observations from MISR (Multi-angle Imaging SpectroRadiometer) and MODIS (Moderate resolution Imaging Spectroradiometer). Relationships between aerosol property trends and air pollutant emission changes are examined. We find that annual mean AOD shows pronounced decreasing trends over EUS and WEU regions, as a result of considerable emission reductions in all major pollutants except for mineral dust and ammonia (NH3). Over the ECC region, AOD increases before 2006 due to emission increases induced by rapid economic development, fluctuates between 2006 and 2011, and subsequently decreases after 2011 in conjunction with effective emission reduction in anthropogenic primary aerosols, sulfur dioxide (SO2), and nitrogen oxides (NOx). The fraction of small-size AOD (<0.7 μm diameter), Ångstrom exponent and single-scattering albedo have generally decreased, while the fractions of large-size (>1.4 μm diameter), nonspherical and absorbing AOD have generally shown increasing trends over EUS and WEU regions, indicating that fine and light-scattering aerosol constituents have been more effectively reduced than coarse and light-absorbing constituents. These trends are consistent with the larger reduction ratios in SO2 and NOx emissions than in primary aerosols, including mineral dust and black carbon (BC

  14. A Comparison of Seasonal and Interannual Variability of Soil Dust Aerosols Over the Atlantic Ocean as Inferred by the Toms AI and AVHRR AOT Retrievals

    NASA Technical Reports Server (NTRS)

    Cakmur, R. V.; Miller, R. L.; Tegen, Ina; Hansen, James E. (Technical Monitor)

    2001-01-01

    The seasonal cycle and interannual variability of two estimates of soil (or 'mineral') dust aerosols are compared: Advanced Very High Resolution Radiometer (AVHRR) aerosol optical thickness (AOT) and Total Ozone Mapping Spectrometer (TOMS) aerosol index (AI), Both data sets, comprising more than a decade of global, daily images, are commonly used to evaluate aerosol transport models. The present comparison is based upon monthly averages, constructed from daily images of each data set for the period between 1984 and 1990, a period that excludes contamination from volcanic eruptions. The comparison focuses upon the Northern Hemisphere subtropical Atlantic Ocean, where soil dust aerosols make the largest contribution to the aerosol load, and are assumed to dominate the variability of each data set. While each retrieval is sensitive to a different aerosol radiative property - absorption for the TOMS AI versus reflectance for the AVHRR AOT - the seasonal cycles of dust loading implied by each retrieval are consistent, if seasonal variations in the height of the aerosol layer are taken into account when interpreting the TOMS AI. On interannual time scales, the correlation is low at most locations. It is suggested that the poor interannual correlation is at least partly a consequence of data availability. When the monthly averages are constructed using only days common to both data sets, the correlation is substantially increased: this consistency suggests that both TOMS and AVHRR accurately measure the aerosol load in any given scene. However, the two retrievals have only a few days in common per month so that these restricted monthly averages have a large uncertainty. Calculations suggest that at least 7 to 10 daily images are needed to estimate reliably the average dust load during any particular month, a threshold that is rarely satisfied by the AVHRR AOT due to the presence of clouds in the domain. By rebinning each data set onto a coarser grid, the availability of

  15. Spatiotemporal variability and contribution of different aerosol types to the Aerosol Optical Depth over the Eastern Mediterranean

    PubMed Central

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos A.; Lelieveld, Jos; Zanis, Prodromos; Pöschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2018-01-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the Aerosol Optical Depth (AOD) over the Eastern Mediterranean as derived from MODIS Terra (3/2000–12/2012) and Aqua (7/2002–12/2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sunphotometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium sized cities, industrial zones, and power plant complexes, seasonal variabilities, and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is ~ 0.22 ± 0.19 with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in Central and Eastern Europe, and transport of dust from the Sahara Desert and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine mode natural aerosols account for ~ 51 %, ~ 34 % and ~ 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account ~ 40 %, ~ 34 % and ~ 26 % of the total AOD550 over the sea, based on MODIS Terra and Aqua observations. PMID:29755508

  16. Spatiotemporal variability and contribution of different aerosol types to the aerosol optical depth over the Eastern Mediterranean

    NASA Astrophysics Data System (ADS)

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos A.; Lelieveld, Jos; Zanis, Prodromos; Pöschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2016-11-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the aerosol optical depth (AOD) over the Eastern Mediterranean as derived from MODIS (Moderate Resolution Imaging Spectroradiometer) Terra (March 2000-December 2012) and Aqua (July 2002-December 2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sun photometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium-sized cities, industrial zones and power plant complexes, seasonal variabilities and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is ˜ 0.22 ± 0.19, with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in central and eastern Europe and transport of dust from the Sahara and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine-mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine-mode natural aerosols account for ˜ 51, ˜ 34 and ˜ 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account ˜ 40, ˜ 34 and ˜ 26 % of the total AOD550 over the sea, based on

  17. Spatiotemporal Variability and Contribution of Different Aerosol Types to the Aerosol Optical Depth over the Eastern Mediterranean

    NASA Technical Reports Server (NTRS)

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos A.; Lelieveld, Jos; Zanis, Prodromos; Poeschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2016-01-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the aerosol optical depth (AOD) over the Eastern Mediterranean as derived from MODIS (Moderate Resolution Imaging Spectroradiometer) Terra (March 2000-December 2012) and Aqua (July 2002-December 2012) satellite instruments. For this purpose, a 0.1deg × 0.1deg gridded MODIS dataset was compiled and validated against sun photometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium-sized cities, industrial zones and power plant complexes, seasonal variabilities and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is approx. 0.22 +/- 0.19, with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in central and eastern Europe and transport of dust from the Sahara and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine-mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine-mode natural aerosols account for approx. 51, approx. 34 and approx. 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account approx. 40, approx. 34 and approx. 26 % of

  18. Features of tropospheric and stratospheric dust.

    PubMed

    Elterman, L; Wexler, R; Chang, D T

    1969-05-01

    A series of 119 profiles obtained over New Mexico comprise aerosol attenuation coefficients vs altitude to about 35 km. These profiles show the existence of several features. A surface convective dust layer extending up to about 5 km is seasonally dependent. Also, a turbidity maximum exists below the tropopause. The altitude of an aerosol maximum in the lower stratosphere is located just below that of the minimum temperature. The colder the minimum temperature, the greater is the aerosol content of the layer. This relationship suggests that the 20-km dust layer is due to convection in tropical air and advection to higher latitudes. Computed averages of optical thickness show that abatement of stratospheric dust from the Mt. Agung eruption became evident in April 1964. Results based on seventy-nine profiles characterizing volcanic dust abatement indicate that above 26 km, the aerosol scale height averages 3.75 km. Extrapolating with this scale height, tabulations are developed for uv, visible, and ir attenuation to 50 km. Optical mixing ratios are used to examine the aerosol concentrations at various altitudes, including a layer at 26 km having an optical thickness 10(-3) for 0.55-micro wavelength.

  19. An aerosol climatology for a rapidly growing arid region (southern Arizona): Major aerosol species and remotely sensed aerosol properties

    NASA Astrophysics Data System (ADS)

    Sorooshian, Armin; Wonaschütz, Anna; Jarjour, Elias G.; Hashimoto, Bryce I.; Schichtel, Bret A.; Betterton, Eric A.

    2011-10-01

    This study reports a comprehensive characterization of atmospheric aerosol particle properties in relation to meteorological and back trajectory data in the southern Arizona region, which includes two of the fastest growing metropolitan areas in the United States (Phoenix and Tucson). Multiple data sets (MODIS, AERONET, OMI/TOMS, MISR, GOCART, ground-based aerosol measurements) are used to examine monthly trends in aerosol composition, aerosol optical depth (AOD), and aerosol size. Fine soil, sulfate, and organics dominate PM2.5 mass in the region. Dust strongly influences the region between March and July owing to the dry and hot meteorological conditions and back trajectory patterns. Because monsoon precipitation begins typically in July, dust levels decrease, while AOD, sulfate, and organic aerosol reach their maximum levels because of summertime photochemistry and monsoon moisture. Evidence points to biogenic volatile organic compounds being a significant source of secondary organic aerosol in this region. Biomass burning also is shown to be a major contributor to the carbonaceous aerosol budget in the region, leading to enhanced organic and elemental carbon levels aloft at a sky-island site north of Tucson (Mt. Lemmon). Phoenix exhibits different monthly trends for aerosol components in comparison with the other sites owing to the strong influence of fossil carbon and anthropogenic dust. Trend analyses between 1988 and 2009 indicate that the strongest statistically significant trends are reductions in sulfate, elemental carbon, and organic carbon, and increases in fine soil during the spring (March-May) at select sites. These results can be explained by population growth, land-use changes, and improved source controls.

  20. Monitoring An Intensive Dust Event over Northern China Using Multi-satellite Observation

    NASA Astrophysics Data System (ADS)

    She, L.; Xue, Y.; Guang, J.; Mei, L.; Che, Y.; Fan, C.; Xie, Y.

    2017-12-01

    The deserts in western/northern China are one of the major mineral dust source regions of the world. Large amount of dust are emitted and blown east and southeast, especially in spring. An intensive dust event occurred over Northern China during May 3 - 8, 2017. The dust storms came from deserts in China and Mongolia. Due to the long-distance transport, more than ten provinces were affected by this dust event, several provinces occurred strong dust storm. In this study, multi-satellite data were employed to analyse the spatial-temporal evolution and dynamic transport behaviour of the dust plume, especially the geostationary satellite data - Himawari8 Advanced Himawari Imager (AHI) data. AHI data was used to estimate hourly Aerosol Optical Depth (AOD) to monitoring the aerosol distribution as well as the dust plume movements, as the dust storms often characterized by high AOD. A simple dust index was also calculated based on AHI VIS and TIR data to estimate the dust intensity. Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data and the Ozone Monitoring Instrument (OMI) Aerosol Index were used as additional data sources to monitor the dust vertical distribution and provide independent information of dust presence. MODIS aerosol product and AERONET aerosol measurements were compared with the AHI retrieved AODs, the comparisons show a good agreement. The dust index was compared with the ground measurements as well as the corresponding RGB image. Simulations from HYSPLIT back-trajectory analysis shows similar temporal variation with the calculated AOD and dust index of the dust plume. Those comparisons with other satellite products and ground measurements suggested both the calculated AOD and dust index well depicted the dust events compared.

  1. Modeling the Interaction of Mineral Dust with Solar Radiation: Spherical versus Non-spherical Particles

    NASA Astrophysics Data System (ADS)

    Hoshyaripour, A.; Vogel, B.; Vogel, H.

    2017-12-01

    Mineral dust, emitted from arid and semi-arid regions, is the most dominant atmospheric aerosol by mass. Beside detrimental effect on air quality, airborne dust also influences the atmospheric radiation by absorbing and scattering solar and terrestrial radiation. As a result, while the long-term radiative impacts of dust are important for climate, the short-term effects are significant for the photovoltaic energy production. Therefore, it is a vital requirement to accurately forecast the effects of dust on energy budget of the atmosphere and surface. To this end, a major issue is the fact that dust particles are non-spherical. Thus, the optical properties of such particles cannot be calculated precisely using the conventional methods like Mie theory that are often used in climate and numerical weather forecast models. In this study, T-Matrix method is employed, which is able to treat the non-sphericity of particles. Dust particles are assumed to be prolate spheroids with aspect ratio of 1.5 distributed in three lognormal modes. The wavelength-dependent refractive indices of dust are used in T-Matrix algorithm to calculate the extinction coefficient, single scattering albedo, asymmetry parameter and backscattering ratio at different wavelengths. These parameters are then implemented in ICON-ART model (ICOsahedral Nonhydrostatic model with Aerosols and Reactive Trace gases) to conduct a global simulation with 80 km horizontal resolution and 90 vertical levels. April 2014 is selected as the simulation period during which North African dust plumes reached central Europe and Germany. Results show that treatment of non-sphericity reduces the dust AOD in the range of 10 to 30%/. The impacts on diffuse and direct radiation at global, regional and local scales show strong dependency on the size distribution of the airborne dust. The implications for modeling and remote sensing the dust impacts on solar energy are also discussed.

  2. Impacts of absorbing aerosol deposition on snowpack and hydrologic cycle in the Rocky Mountain region using variable-resolution CESM (VR-CESM)

    NASA Astrophysics Data System (ADS)

    Wu, C.; Liu, X.; Lin, Z.; Rahimi-Esfarjani, S. R.; Lu, Z.

    2017-12-01

    Deposition of light-absorbing aerosols (LAAs) including black carbon (BC) and dust onto snow surface has been suggested to reduce the snow albedo, and modulate the snowpack and consequent hydrologic cycle. In this study we use the variable-resolution Community Earth System Model (VR-CESM) to quantify the impacts of LAAs deposition onto snow in the Rocky Mountain region (RMR) during the period of 1981-2005. We first evaluate the model simulation of LAA concentrations both in the atmosphere and in snow, and then investigate the snowpack and runoff changes induced by LAAs-in-snow. The model simulates similar magnitudes of surface atmospheric dust concentrations as observations, but underestimates surface atmospheric BC concentrations by about a factor of two. Despite of this, the magnitude of BC-in-snow concentrations is overall comparable to observations. Regional mean surface radiative effect (SRE) due to LAAs-in-snow reaches up to 0.6-1.7 W m-2 in spring, and dust contributes to about 21-43% of total SRE. Maximum surface air temperature increase due to the LLA's SRE is around 0.9-1.1oC. Snow water equivalent and snow cover fraction reduce by around 2-50 mm and 0.05-0.2, respectively in the two regions around the mountains (Eastern Snake River Plain and Southwestern Wyoming) due to positive snow-albedo feedbacks. During the snow melting period, LAAs accelerate the hydrologic cycle with runoff increased by 7%-42% in April-May and reduced by 2-23% in June-July in the mountainous regions. Under the influence of LAAs-in-snow, Southern Rockies experience the most significant reduction of runoff by about 15% in the later stage of snow melt (i.e., June-July). Our results highlight the potentially important role of LAAs-in-snow in the historical and future changes of snowpack in the RMR.

  3. An Analysis of AERONET Aerosol Absorption Properties and Classifications Representative of Aerosol Source Regions

    NASA Technical Reports Server (NTRS)

    Giles, David M.; Holben, Brent N.; Eck, Thomas F.; Sinyuk, Aliaksandr; Smirnov, Alexander; Slutsker, Ilya; Dickerson, R. R.; Thompson, A. M.; Schafer, J. S.

    2012-01-01

    Partitioning of mineral dust, pollution, smoke, and mixtures using remote sensing techniques can help improve accuracy of satellite retrievals and assessments of the aerosol radiative impact on climate. Spectral aerosol optical depth (tau) and single scattering albedo (omega (sub 0) ) from Aerosol Robotic Network (AERONET) measurements are used to form absorption [i.e., omega (sub 0) and absorption Angstrom exponent (alpha(sub abs))] and size [i.e., extinction Angstrom exponent (alpha(sub ext)) and fine mode fraction of tau] relationships to infer dominant aerosol types. Using the long-term AERONET data set (1999-2010), 19 sites are grouped by aerosol type based on known source regions to: (1) determine the average omega (sub 0) and alpha(sub abs) at each site (expanding upon previous work); (2) perform a sensitivity study on alpha(sub abs) by varying the spectral omega (sub 0); and (3) test the ability of each absorption and size relationship to distinguish aerosol types. The spectral omega (sub 0) averages indicate slightly more aerosol absorption (i.e., a 0.0 < delta omega (sub 0) <= 0.02 decrease) than in previous work and optical mixtures of pollution and smoke with dust show stronger absorption than dust alone. Frequency distributions of alpha(sub abs) show significant overlap among aerosol type categories and at least 10% of the alpha(sub abs) retrievals in each category are below 1.0. Perturbing the spectral omega (sub 0) by +/- 0.03 induces significant alpha(sub abs) changes from the unperturbed value by at least approx. +/- 0.6 for Dust, approx. +/-0.2 for Mixed, and approx. +/-0.1 for Urban/Industrial and Biomass Burning. The omega (sub 0)440nm and alpha(sub ext) 440-870nm relationship shows the best separation among aerosol type clusters, providing a simple technique for determining aerosol type from surface- and future space-based instrumentation.

  4. Modeling analysis of secondary inorganic aerosols over China: pollution characteristics, and meteorological and dust impacts.

    PubMed

    Fu, Xiao; Wang, Shuxiao; Chang, Xing; Cai, Siyi; Xing, Jia; Hao, Jiming

    2016-10-26

    Secondary inorganic aerosols (SIA) are the predominant components of fine particulate matter (PM 2.5 ) and have significant impacts on air quality, human health, and climate change. In this study, the Community Multiscale Air Quality modeling system (CMAQ) was modified to incorporate SO 2 heterogeneous reactions on the surface of dust particles. The revised model was then used to simulate the spatiotemporal characteristics of SIA over China and analyze the impacts of meteorological factors and dust on SIA formation. Including the effects of dust improved model performance for the simulation of SIA concentrations, particularly for sulfate. The simulated annual SIA concentration in China was approximately 10.1 μg/m 3 on domain average, with strong seasonal variation: highest in winter and lowest in summer. High SIA concentrations were concentrated in developed regions with high precursor emissions, such as the North China Plain, Yangtze River Delta, Sichuan Basin, and Pearl River Delta. Strong correlations between meteorological factors and SIA pollution levels suggested that heterogeneous reactions under high humidity played an important role on SIA formation, particularly during severe haze pollution periods. Acting as surfaces for heterogeneous reactions, dust particles significantly affected sulfate formation, suggesting the importance of reducing dust emissions for controlling SIA and PM 2.5 pollution.

  5. Modeling analysis of secondary inorganic aerosols over China: pollution characteristics, and meteorological and dust impacts

    NASA Astrophysics Data System (ADS)

    Fu, Xiao; Wang, Shuxiao; Chang, Xing; Cai, Siyi; Xing, Jia; Hao, Jiming

    2016-10-01

    Secondary inorganic aerosols (SIA) are the predominant components of fine particulate matter (PM2.5) and have significant impacts on air quality, human health, and climate change. In this study, the Community Multiscale Air Quality modeling system (CMAQ) was modified to incorporate SO2 heterogeneous reactions on the surface of dust particles. The revised model was then used to simulate the spatiotemporal characteristics of SIA over China and analyze the impacts of meteorological factors and dust on SIA formation. Including the effects of dust improved model performance for the simulation of SIA concentrations, particularly for sulfate. The simulated annual SIA concentration in China was approximately 10.1 μg/m3 on domain average, with strong seasonal variation: highest in winter and lowest in summer. High SIA concentrations were concentrated in developed regions with high precursor emissions, such as the North China Plain, Yangtze River Delta, Sichuan Basin, and Pearl River Delta. Strong correlations between meteorological factors and SIA pollution levels suggested that heterogeneous reactions under high humidity played an important role on SIA formation, particularly during severe haze pollution periods. Acting as surfaces for heterogeneous reactions, dust particles significantly affected sulfate formation, suggesting the importance of reducing dust emissions for controlling SIA and PM2.5 pollution.

  6. Modeling analysis of secondary inorganic aerosols over China: pollution characteristics, and meteorological and dust impacts

    PubMed Central

    Fu, Xiao; Wang, Shuxiao; Chang, Xing; Cai, Siyi; Xing, Jia; Hao, Jiming

    2016-01-01

    Secondary inorganic aerosols (SIA) are the predominant components of fine particulate matter (PM2.5) and have significant impacts on air quality, human health, and climate change. In this study, the Community Multiscale Air Quality modeling system (CMAQ) was modified to incorporate SO2 heterogeneous reactions on the surface of dust particles. The revised model was then used to simulate the spatiotemporal characteristics of SIA over China and analyze the impacts of meteorological factors and dust on SIA formation. Including the effects of dust improved model performance for the simulation of SIA concentrations, particularly for sulfate. The simulated annual SIA concentration in China was approximately 10.1 μg/m3 on domain average, with strong seasonal variation: highest in winter and lowest in summer. High SIA concentrations were concentrated in developed regions with high precursor emissions, such as the North China Plain, Yangtze River Delta, Sichuan Basin, and Pearl River Delta. Strong correlations between meteorological factors and SIA pollution levels suggested that heterogeneous reactions under high humidity played an important role on SIA formation, particularly during severe haze pollution periods. Acting as surfaces for heterogeneous reactions, dust particles significantly affected sulfate formation, suggesting the importance of reducing dust emissions for controlling SIA and PM2.5 pollution. PMID:27782166

  7. Niamey Dust Observations

    DOE Data Explorer

    Flynn, Connor

    2008-10-01

    Niamey aerosol are composed of two main components: dust due to the proximity of the Sahara Desert, and soot from local and regional biomass burning. The purpose of this data product is to identify when the local conditions are dominated by the dust component so that the properties of the dust events can be further studied.

  8. Types, Sizes, Shapes and Distributions of Mars Ice and Dust Aerosols from the MGS TES Emission Phase Function Observations

    NASA Astrophysics Data System (ADS)

    Clancy, R. T.; Wolff, M. J.; Christensen, P. R.

    2001-12-01

    A full Mars year (1999-2001) of emission phase function (EPF observations from Mars Global Surveyor (MGS) Thermal Emission Spectrometer (TES) provide the most complete study of Mars dust and ice aerosol properties to date. TES visible (solar band average) and infrared spectral (6-30 micron, 10 invcm res) EPF sequences are analyzed self-consistently with detailed multiple scattering radiative transfer (RT) codes to obtain first-time seasonal/latitudinal distributions of aerosol visible optical depths, particle sizes, and single scattering phase functions. As a consequence of the combined angular and wavelength coverage, we are able to define two distinct ice cloud types at 45S-45N latitudes on Mars. Type 1 ice clouds exhibit small particle sizes (1-2 micron radii), as well as a broad, deep minimum in side scattering indicative of aligned ice grains (see Wolff et al., 2001). Type 1 ice aerosols are most prevalent in the southern hemisphere during Mars aphelion, but also appear more widely distributed in season and latitude as topographic and high altitude (above 20 km) ice hazes. Type 2 ice clouds exhibit larger particle sizes (2-4 microns) and a much narrower side-scattering minimum, indicative of poorer grain alignment or a change in particle shape relative to the type 1 ice clouds (see Wolff et al., 2001). Type 2 ice clouds appear most prominently in the northern subtropical aphelion cloud belt, where relatively low altitudes of water vapor saturation (10 km) coincide with strong advective transport (Clancy et al., 1996). Retrieved dust particle radii of 1.5-1.8 micron are consistent with Pathfinder (Tomasko et al., 1999) and recent Viking/Mariner 9 reanalyses (e.g., size distribution B of Clancy et al., 1995). Detailed spectral modeling of the solar passband also implies agreement of EPF-derived dust single scattering albedos (ssa) with the ssa results from Tomasko et al.(table 8 therein). Spatial and seasonal changes in the dust ssa (0.92-0.95, solar band

  9. The Size Distribution of Atmospheric Aerosols at Kosan, Korea during ACE-Asia: Changes due to Dust Input and Scavenging by Precipitation

    NASA Astrophysics Data System (ADS)

    Jung, C.; Kim, J.; Choi, B.; Brechtel, F. J.; Buzorius, G.; Oh, S.

    2001-12-01

    Measurements of size-resolved aerosol number concentrations were made at the Kosan supersite in Korea during the ACE-Asia intensive observation period. An optical particle counter (OPC) was used for measurements in the 0.3-25.0 micrometer diameter size range every ten minutes while a scanning electrical mobility spectrometer (SEMS) was used for smaller particles. A comparison of size distributions between dust and non-dust input periods and times with and without precipitation has been performed. During dust events, the number and volume concentrations of large particles (>1.35 micrometer) increased by factors of 10 and 1000, respectively. Also, a dominant number mode diameter between 2.23-3.67 micrometer was observed during dust events. The number concentrations of smaller particles observed by the OPC (0.3-1 micrometer) and SEMS (0.005-0.6 micrometer) were relatively smaller during dust events, consistent with previous studies and the effect of coagulation processes (Zaizen et al., 1995; Chun et al., 2001). During precipitation events, coarse mode particles (>1 micrometer) were scavenged more efficiently than smaller particles. This result suggests that large particles are efficiently scavenged by impaction with raindrops. In contrast, relatively minor reductions in the number concentrations of small particles (0.3-1 micrometer) were observed during precipitation events. SEMS results during one precipitation event indicate factor of three reductions in total number and area concentrations for particle sizes below the detection limit of the OPC. Results from theoretical analyses of scavenging rates as a function of particle size during precipitation events will be presented and compared to values derived from observed size distributions. References Chun, Y., Kim, J., Choi, J. C., Boo, K. O., Oh, S. N., and Lee, M. (2001). Characteristic number size distribution of aerosol during Asian dust period in Korea, Atmospheric Environment, 35, 2715-2721. Zaizen, Y

  10. Application of AERONET Single Scattering Albedo and Absorption Angstrom Exponent to Classify Dominant Aerosol Types during DRAGON Campaigns

    NASA Astrophysics Data System (ADS)

    Giles, D. M.; Holben, B. N.; Eck, T. F.; Schafer, J.; Crawford, J. H.; Kim, J.; Sano, I.; Liew, S.; Salinas Cortijo, S. V.; Chew, B. N.; Lim, H.; Smirnov, A.; Sorokin, M.; Kenny, P.; Slutsker, I.

    2013-12-01

    Aerosols can have major implications on human health by inducing respiratory diseases due to inhalation of fine particles from biomass burning smoke or industrial pollution and on radiative forcing whereby the presence of absorbing aerosol particles (e.g., black carbon) increases atmospheric heating. Aerosol classification techniques have utilized aerosol loading and aerosol properties derived from multi-spectral and multi-angle observations by ground-based (e.g., AERONET) and satellite instrumentation (e.g., MISR). Aerosol Robotic Network (AERONET) data have been utilized to determine aerosol types by implementing various combinations of measured aerosol optical depth or retrieved size and absorption aerosol properties (e.g., Gobbi et al., 2007; Russell et al., 2010). Giles et al. [2012] showed single scattering albedo (SSA) relationship with extinction Angstrom exponent (EAE) can provide an estimate of the general classification of dominant aerosol types (i.e., desert dust, urban/industrial pollution, biomass burning smoke, and mixtures) based on data from ~20 AERONET sites located in known aerosol source regions. In addition, the absorption Angstrom exponent relationship with EAE can provide an indication of the dominant absorbing aerosol type such as dust, black carbon, brown carbon, or mixtures of them. These classification techniques are applied to the AERONET Level 2.0 quality assured data sets collected during Distributed Regional Aerosol Gridded Observational Network (DRAGON) campaigns in Maryland (USA), Japan, South Korea, Singapore, Penang (Malaysia), and California (USA). An analysis of aerosol type classification for DRAGON sites is performed as well as an assessment of the spatial variability of the aerosol types for selected DRAGON campaigns. Giles, D. M., B. N. Holben, T. F. Eck, A. Sinyuk, A. Smirnov, I. Slutsker, R. R. Dickerson, A. M. Thompson, and J. S. Schafer (2012), An analysis of AERONET aerosol absorption properties and classifications

  11. Integrative Analysis of Desert Dust Size and Abundance Suggests Less Dust Climate Cooling

    NASA Technical Reports Server (NTRS)

    Kok, Jasper F.; Ridley, David A.; Zhou, Qing; Miller, Ron L.; Zhao, Chun; Heald, Colette L.; Ward, Daniel S.; Albani, Samuel; Haustein, Karsten

    2017-01-01

    Desert dust aerosols affect Earths global energy balance through interactions with radiation, clouds, and ecosystems. But the magnitudes of these effects are so uncertain that it remains unclear whether atmospheric dust has a net warming or cooling effect on global climate. Consequently, it is still uncertain whether large changes in atmospheric dust loading over the past century have slowed or accelerated anthropogenic climate change, and the climate impact of possible future alterations in dust loading is similarly disputed. Here we use an integrative analysis of dust aerosol sizes and abundance to constrain the climatic impact of dust through direct interactions with radiation. Using a combination of observational, experimental, and model data, we find that atmospheric dust is substantially coarser than represented in current climate models. Since coarse dust warms global climate, the dust direct radiative effect (DRE) is likely less cooling than the 0.4 W m superscript 2 estimated by models in a current ensemble. We constrain the dust DRE to -0.20 (-0.48 to +0.20) W m superscript 2, which suggests that the dust DRE produces only about half the cooling that current models estimate, and raises the possibility that dust DRE is actually net warming the planet.

  12. The effect of smoke, dust, and pollution aerosol on shallow cloud development over the Atlantic Ocean

    PubMed Central

    Kaufman, Yoram J.; Koren, Ilan; Remer, Lorraine A.; Rosenfeld, Daniel; Rudich, Yinon

    2005-01-01

    Clouds developing in a polluted environment tend to have more numerous but smaller droplets. This property may lead to suppression of precipitation and longer cloud lifetime. Absorption of incoming solar radiation by aerosols, however, can reduce the cloud cover. The net aerosol effect on clouds is currently the largest uncertainty in evaluating climate forcing. Using large statistics of 1-km resolution MODIS (Moderate Resolution Imaging Spectroradiometer) satellite data, we study the aerosol effect on shallow water clouds, separately in four regions of the Atlantic Ocean, for June through August 2002: marine aerosol (30°S–20°S), smoke (20°S–5°N), mineral dust (5°N–25°N), and pollution aerosols (30°N– 60°N). All four aerosol types affect the cloud droplet size. We also find that the coverage of shallow clouds increases in all of the cases by 0.2–0.4 from clean to polluted, smoky, or dusty conditions. Covariability analysis with meteorological parameters associates most of this change to aerosol, for each of the four regions and 3 months studied. In our opinion, there is low probability that the net aerosol effect can be explained by coincidental, unresolved, changes in meteorological conditions that also accumulate aerosol, or errors in the data, although further in situ measurements and model developments are needed to fully understand the processes. The radiative effect at the top of the atmosphere incurred by the aerosol effect on the shallow clouds and solar radiation is –11 ± 3 W/m2 for the 3 months studied; 2/3 of it is due to the aerosol-induced cloud changes, and 1/3 is due to aerosol direct radiative effect. PMID:16076949

  13. On the visibility of airborne volcanic ash and mineral dust

    NASA Astrophysics Data System (ADS)

    Weinzierl, B.; Sauer, D. N.; Minikin, A.; Reitebuch, O.; Dahlkötter, F.; Mayer, B. C.; Emde, C.; Tegen, I.; Gasteiger, J.; Petzold, A.; Veira, A.; Kueppers, U.; Schumann, U.

    2012-12-01

    After the eruption of the Eyjafjalla volcano (Iceland) in April 2010 which caused the most extensive restrictions of the airspace over Europe since the end of World War II, the aviation safety concept of avoiding "visible ash", i.e. volcanic ash that can be seen by the human eye, was recommended. However so far, no clear definition of "visible ash" and no relation between the visibility of an aerosol layer and related aerosol mass concentrations are available. The goal of our study is to assess whether it is possible from the pilot's perspective in flight to detect the presence of volcanic ash and to distinguish between volcanic ash and other aerosol layers just by sight. In our presentation, we focus the comparison with other aerosols on aerosol types impacting aviation: Besides volcanic ash, dust storms are known to be avoided by aircraft. We use in-situ and lidar data as well photographs taken onboard the DLR research aircraft Falcon during the Saharan Mineral Dust Experiments (SAMUM) in 2006 and 2008 and during the Eyjafjalla volcanic eruption in April/May 2010. We complement this analysis with numerical modelling, using idealized radiative transfer simulations with the 3D Monte Carlo radiative transfer code MYSTIC for a variety of selected viewing geometries. Both aerosol types, Saharan mineral dust and volcanic ash, show an enhanced coarse mode (> 1 μm) aerosol concentration, but volcanic ash aerosol additionally contains a significant number of Aitken mode particles (< 150 nm). Volcanic ash is slightly more absorbing than mineral dust, and the spectral behaviour of the refractive index is slightly different. According to our simulations, these differences are not detectable just by human eye. Furthermore, our data show, that it is difficult to define a lower threshold for the visibility of an aerosol layer because the visual detectability depends on many parameters, including the thickness of the aerosol layer, the brightness and color contrast between the

  14. Detection of anthropogenic dust using CALIPSO lidar measurements

    NASA Astrophysics Data System (ADS)

    Huang, J.; Liu, J.; Chen, B.; Nasiri, S. L.

    2015-04-01

    Anthropogenic dusts are those produced by human activities on disturbed soils, which are mainly cropland, pasture, and urbanized regions and are a subset of the total dust load which includes natural sources from desert regions. Our knowledge of anthropogenic dusts is still very limited due to a lack of data on source distribution and magnitude, and on their effect on radiative forcing which may be comparable to other anthropogenic aerosols. To understand the contribution of anthropogenic dust to the total global dust load and its effect on radiative transfer and climate, it is important to identify them from total dust. In this study, a new technique for distinguishing anthropogenic dust from natural dust is proposed by using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) dust and planetary boundary layer (PBL) height retrievals along with a land use dataset. Using this technique, the global distribution of dust is analyzed and the relative contribution of anthropogenic and natural dust sources to regional and global emissions are estimated. Results reveal that local anthropogenic dust aerosol due to human activity, such as agriculture, industrial activity, transportation, and overgrazing, accounts for about 25% of the global continental dust load. Of these anthropogenic dust aerosols, more than 53% come from semi-arid and semi-wet regions. Annual mean anthropogenic dust column burden (DCB) values range from 0.42 g m-2 with a maximum in India to 0.12 g m-2 with a minimum in North America. A better understanding of anthropogenic dust emission will enable us to focus on human activities in these critical regions and with such knowledge we will be better able to improve global dust models and to explore the effects of anthropogenic emission on radiative forcing, climate change and air quality in the future.

  15. North Atlantic Aerosol Radiative Impacts Based on Satellite Measurements and Aerosol Intensive Properties from TARFOX and ACE-2

    NASA Technical Reports Server (NTRS)

    Bergstrom, Robert A.; Russell, Philip B.

    2000-01-01

    We estimate the impact of North Atlantic aerosols on the net shortwave flux at the tropopause by combining maps of satellite-derived aerosol optical depth (AOD) with model aerosol properties. We exclude African dust, primarily by restricting latitudes to 25-60 N. Aerosol properties were determined via column closure analyses in two recent experiments, TARFOX and ACE 2. The analyses use in situ measurements of aerosol composition and air- and ship-borne sunphotometer measurements of AOD spectra. The resulting aerosol model yields computed flux sensitivities (dFlux/dAOD) that agree with measurements by airborne flux radiometers in TARFOX. It has a midvisible single- scattering albedo of 0.9, which is in the range obtained from in situ measurements of aerosol scattering and absorption in both TARFOX and ACE 2. Combining seasonal maps of AVHRR-derived midvisible AOD with the aerosol model yields maps of 24-hour average net radiative flux changes at the tropopause. For cloud-free conditions, results range from -9 W/sq m near the eastern US coastline in the summer to -1 W/sq m in the mid-Atlantic during winter; the regional annual average is -3.5 W/sq m. Using a non- absorbing aerosol model increases these values by about 30%. We estimate the effect of clouds using ISCCP cloud-fraction maps. Because ISCCP midlatitude North Atlantic cloud fractions are relatively large, they greatly reduce the computed aerosol-induced flux changes. For example, the regional annual average decreases from -3.5 W/sq m to -0.8 W/sq m. We compare results to previous model calculations for a variety of aerosol types.

  16. North Atlantic Aerosol Radiative Effects Based on Satellite Measurements and Aerosol Intensive Properties from TARFOX and ACE-2

    NASA Technical Reports Server (NTRS)

    Bergstrom, Robert W.; Russell, Philip B.

    2000-01-01

    We estimate the impact of North Atlantic aerosols on the net shortwave flux at the tropopause by combining maps of satellite-derived aerosol optical depth (AOD) with model aerosol properties. We exclude African dust, primarily by restricting latitudes to 25-60 N. Aerosol properties were determined via column closure analyses in two recent experiments, TARFOX and ACE 2. The analyses use in situ measurements of aerosol composition and air- and ship-borne sunphotometer measurements of AOD spectra. The resulting aerosol model yields computed flux sensitivities (dFlux/dAOD) that agree with measurements by airborne flux radiometers in TARFOX. It has a midvisible single-scattering albedo of 0.9, which is in the range obtained from in situ measurements of aerosol scattering and absorption in both TARFOX and ACE 2. Combining seasonal maps of AVHRR-derived midvisible AOD with the aerosol model yields maps of 24-hour average net radiative flux changes at the tropopause. For cloud-free conditions, results range from -9 W/sq m near the eastern US coastline in the summer to -1 W/sq m in the mid-Atlantic during winter; the regional annual average is -3.5 W/sq m. Using a non- absorbing aerosol model increases these values by about 30%. We estimate the effect of clouds using ISCCP cloud-fraction maps. Because ISCCP midlatitude North Atlantic cloud fractions are relatively large, they greatly reduce the computed aerosol-induced flux changes. For example, the regional annual average decreases from -3.5 W/sq m to -0.8 W/sq m. We compare results to previous model calculations for a variety of aerosol types.

  17. North Atlantic Aerosol Radiative Impacts Based on Satellite Measurements and Aerosol Intensive Properties from TARFOX and ACE-2

    NASA Technical Reports Server (NTRS)

    Russell, Philip B.; Bergstrom, Robert W.; Schmid, Beat; Livingston, John M.

    2000-01-01

    We estimate the impact of North Atlantic aerosols on the net shortwave flux at the tropopause by combining maps of satellite-derived aerosol optical depth (AOD) with model aerosol properties. We exclude African dust, primarily by restricting latitudes to 25-60 N. Aerosol properties were determined via column closure analyses in two recent experiments, TARFOX and ACE 2. The analyses use in situ measurements of aerosol composition and air- and ship-borne sunphotometer measurements of AOD spectra. The resulting aerosol model yields computed flux sensitivities (dFlux/dAOD) that agree with measurements by airborne flux radiometers in TARFOX. It has a midvisible single-scattering albedo of 0.9, which is in the range obtained from in situ measurements of aerosol scattering and absorption in both TARFOX and ACE 2. Combining seasonal maps of AVHRR-derived midvisible AOD with the aerosol model yields maps of 24-hour average net radiative flux changes at the tropopause. For cloud-free conditions, results range from -9 W/sq m near the eastern US coastline in the summer to -1 W/sq m in the mid-Atlantic during winter; the regional annual average is -3.5 W/sq m. Using a non- absorbing aerosol model increases these values by about 30%. We estimate the effect of clouds using ISCCP cloud-fraction maps. Because ISCCP midlatitude North Atlantic cloud fractions are relatively large, they greatly reduce the computed aerosol-induced flux changes. For example, the regional annual average decreases from -3.5 W/sq m to -0.8 W/sq m. We compare results to previous model calculations for a variety of aerosol types.

  18. The Size of Dust and Smoke

    NASA Technical Reports Server (NTRS)

    2005-01-01

    Desert dust particles tend to be larger in size than aerosols that originate from the processes of combustion. How precisely do the size of the aerosol particles comprising the dust that obscured the Red Sea on July 26, 2005, contrast with the size of the haze particles that obscured the United States eastern seaboard on the same day? NASA's Multi-angle Imaging SpectroRadiometer (MISR), which views Earth at nine different angles in four wavelengths, provides information about the amount, size, and shape of airborne particles. Here, MISR aerosol amount and size is presented for these two events. These MISR results distinguish desert dust, the most common non-spherical aerosol type, from pollution and forest fire particles. Determining aerosol characteristics is a key to understanding how aerosol particles influence the size, abundance, and rate of production of cloud droplets, and to a better understanding of how aerosols influence clouds and climate.

    The left panel of each of these two image sets (Red Sea, left; U.S. coastline, right) is a natural-color view from MISR's 70-degree forward viewing camera. The color-coded maps in the central panels show aerosol optical depth; the right panels provide a measure of aerosol size, expressed as the 'Angstrom exponent.' For the optical depth maps, yellow pixels indicate the most optically-thick aerosols, whereas the red, green and blue pixels represent progressively decreasing aerosol amounts. For this dramatic dust storm over the Red Sea, the aerosol is quite thick, and in some places, the dust over water is too optically thick for MISR to retrieve the aerosol amount. For the eastern seaboard haze, the thickest aerosols have accumulated over the Atlantic Ocean off the coasts of South Carolina and Georgia. Cases where no successful retrieval occurred, either due to extremely high aerosol optical thickness or to clouds, appear as dark gray pixels.

    For the Angstrom exponent maps, the blue and green pixels

  19. The physics of wind-blown sand and dust

    NASA Astrophysics Data System (ADS)

    Kok, Jasper F.; Parteli, Eric J. R.; Michaels, Timothy I.; Karam, Diana Bou

    2012-10-01

    The transport of sand and dust by wind is a potent erosional force, creates sand dunes and ripples, and loads the atmosphere with suspended dust aerosols. This paper presents an extensive review of the physics of wind-blown sand and dust on Earth and Mars. Specifically, we review the physics of aeolian saltation, the formation and development of sand dunes and ripples, the physics of dust aerosol emission, the weather phenomena that trigger dust storms, and the lifting of dust by dust devils and other small-scale vortices. We also discuss the physics of wind-blown sand and dune formation on Venus and Titan.

  20. The physics of wind-blown sand and dust.

    PubMed

    Kok, Jasper F; Parteli, Eric J R; Michaels, Timothy I; Karam, Diana Bou

    2012-10-01

    The transport of sand and dust by wind is a potent erosional force, creates sand dunes and ripples, and loads the atmosphere with suspended dust aerosols. This paper presents an extensive review of the physics of wind-blown sand and dust on Earth and Mars. Specifically, we review the physics of aeolian saltation, the formation and development of sand dunes and ripples, the physics of dust aerosol emission, the weather phenomena that trigger dust storms, and the lifting of dust by dust devils and other small-scale vortices. We also discuss the physics of wind-blown sand and dune formation on Venus and Titan.

  1. Evaluating the impact of above-cloud aerosols on cloud optical depth retrievals from MODIS

    NASA Astrophysics Data System (ADS)

    Alfaro, Ricardo

    Using two different operational Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) cloud optical depth (COD) retrievals (visible and shortwave infrared), the impacts of above-cloud absorbing aerosols on the standard COD retrievals are evaluated. For fine-mode aerosol particles, aerosol optical depth (AOD) values diminish sharply from the visible to the shortwave infrared channels. Thus, a suppressed above-cloud particle radiance aliasing effect occurs for COD retrievals using shortwave infrared channels. Aerosol Index (AI) from the spatially and temporally collocated Ozone Monitoring Instrument (OMI) are used to identify above-cloud aerosol particle loading over the southern Atlantic Ocean, including both smoke and dust from the African sub-continent. MODIS and OMI Collocated Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) data are used to constrain cloud phase and provide contextual above-cloud AOD values. The frequency of occurrence of above-cloud aerosols is depicted on a global scale for the spring and summer seasons from OMI and CALIOP, thus indicating the significance of the problem. Seasonal frequencies for smoke-over-cloud off the southwestern Africa coastline reach 20--50% in boreal summer. We find a corresponding low COD bias of 10--20% for standard MODIS COD retrievals when averaged OMI AI are larger than 1.0. No such bias is found over the Saharan dust outflow region off northern Africa, since both MODIS visible and shortwave in channels are vulnerable to dust particle aliasing, and thus a COD impact cannot be isolated with this method. A similar result is found for a smaller domain, in the Gulf of Tonkin region, from smoke advection over marine stratocumulus clouds and outflow into the northern South China Sea in spring. This study shows the necessity of accounting for the above-cloud aerosol events for future studies using standard MODIS cloud products in biomass burning outflow regions, through the use of

  2. Fine-scale application of WRF-CAM5 during a dust storm episode over East Asia: Sensitivity to grid resolutions and aerosol activation parameterizations

    NASA Astrophysics Data System (ADS)

    Wang, Kai; Zhang, Yang; Zhang, Xin; Fan, Jiwen; Leung, L. Ruby; Zheng, Bo; Zhang, Qiang; He, Kebin

    2018-03-01

    An advanced online-coupled meteorology and chemistry model WRF-CAM5 has been applied to East Asia using triple-nested domains at different grid resolutions (i.e., 36-, 12-, and 4-km) to simulate a severe dust storm period in spring 2010. Analyses are performed to evaluate the model performance and investigate model sensitivity to different horizontal grid sizes and aerosol activation parameterizations and to examine aerosol-cloud interactions and their impacts on the air quality. A comprehensive model evaluation of the baseline simulations using the default Abdul-Razzak and Ghan (AG) aerosol activation scheme shows that the model can well predict major meteorological variables such as 2-m temperature (T2), water vapor mixing ratio (Q2), 10-m wind speed (WS10) and wind direction (WD10), and shortwave and longwave radiation across different resolutions with domain-average normalized mean biases typically within ±15%. The baseline simulations also show moderate biases for precipitation and moderate-to-large underpredictions for other major variables associated with aerosol-cloud interactions such as cloud droplet number concentration (CDNC), cloud optical thickness (COT), and cloud liquid water path (LWP) due to uncertainties or limitations in the aerosol-cloud treatments. The model performance is sensitive to grid resolutions, especially for surface meteorological variables such as T2, Q2, WS10, and WD10, with the performance generally improving at finer grid resolutions for those variables. Comparison of the sensitivity simulations with an alternative (i.e., the Fountoukis and Nenes (FN) series scheme) and the default (i.e., AG scheme) aerosol activation scheme shows that the former predicts larger values for cloud variables such as CDNC and COT across all grid resolutions and improves the overall domain-average model performance for many cloud/radiation variables and precipitation. Sensitivity simulations using the FN series scheme also have large impacts on

  3. Optical properties of mineral dust aerosol including analysis of particle size, composition, and shape effects, and the impact of physical and chemical processing

    NASA Astrophysics Data System (ADS)

    Alexander, Jennifer Mary

    Atmospheric mineral dust has a large impact on the earth's radiation balance and climate. The radiative effects of mineral dust depend on factors including, particle size, shape, and composition which can all be extremely complex. Mineral dust particles are typically irregular in shape and can include sharp edges, voids, and fine scale surface roughness. Particle shape can also depend on the type of mineral and can vary as a function of particle size. In addition, atmospheric mineral dust is a complex mixture of different minerals as well as other, possibly organic, components that have been mixed in while these particles are suspended in the atmosphere. Aerosol optical properties are investigated in this work, including studies of the effect of particle size, shape, and composition on the infrared (IR) extinction and visible scattering properties in order to achieve more accurate modeling methods. Studies of particle shape effects on dust optical properties for single component mineral samples of silicate clay and diatomaceous earth are carried out here first. Experimental measurements are modeled using T-matrix theory in a uniform spheroid approximation. Previous efforts to simulate the measured optical properties of silicate clay, using models that assumed particle shape was independent of particle size, have achieved only limited success. However, a model which accounts for a correlation between particle size and shape for the silicate clays offers a large improvement over earlier modeling approaches. Diatomaceous earth is also studied as an example of a single component mineral dust aerosol with extreme particle shapes. A particle shape distribution, determined by fitting the experimental IR extinction data, used as a basis for modeling the visible light scattering properties. While the visible simulations show only modestly good agreement with the scattering data, the fits are generally better than those obtained using more commonly invoked particle shape

  4. Characterisation of bio-aerosols during dust storm period in N-NW India

    NASA Astrophysics Data System (ADS)

    Yadav, Sudesh; Chauhan, M. S.; Sharma, Anupam

    Bio-investigations for pollen and spores were performed on dry free-fall dust and PM 10 aerosol samples, collected from three different locations separated by a distance of 600 km, situated in dust storm hit region of N-NW India. Presence of pollen of trees namely Prosopis ( Prosopis juliflora and Prosopis cinearia), Acacia, Syzygium, Pinus, Cedrus, Holoptelea and shrubs namely Ziziphus, Ricinus, Ephedra and members of Fabaceae, Oleaceae families was recorded but with varying proportions in the samples of different locations. Poaceae, Chenopodiaceae/Amaranthaceae, Caryophyllaceae, Brassicaceae and Cyperaceae (sedges) were some of the herb pollen identified in the samples. Among the fungal spores Nigrospora was seen in almost all samples. Nigrospora is a well known allergen and causes health problems. The concentration of trees and shrubs increases in the windward direction just as the climate changes from hot arid to semiarid. The higher frequency of grasses (Poaceae) or herbs could either be a result of the presence of these herbs in the sampling area and hence the higher production of pollen/spores or due to the resuspension from the exposed surface by the high-intensity winds. But we cannot ascertain the exact process at this stage. The overall similarity in the pollen and spore assemblage in our dust samples indicates a common connection or source(s) to the dust in this region. Presence of the pollen of the species of Himalayan origin in our entire samples strongly point towards a Himalayan connection, could be direct or indirect, to the bioaerosols and hence dust in N-NW India. In order to understand the transport path and processes involved therein, present study needs further extension with more number of samples and with reference to meteorological parameters.

  5. Tar balls are processed, weakly absorbing, primary aerosol particles formed downwind of boreal forest fires

    NASA Astrophysics Data System (ADS)

    Sedlacek, A. J., III; Buseck, P. R.; Adachi, K.; Kleinman, L. I.; Onasch, T. B.; Springston, S. R.

    2017-12-01

    Biomass burning is a major source of light-absorbing black and brown carbonaceous aerosols Brown carbon is a poorly characterized mixture that includes tar balls (TBs), a type of carbonaceous particle unique to biomass burning. Here we describe the first atmospheric observations of the formation and evolution of TBs Aerosol particles were collected on TEM grids during individual aircraft transects at varying downwind distances from the Colockum Tarp wildland fire. The TEM images show primary particles transforming from viscous, impact-deformed particles to spherical TBs. The number fraction of TBs in the wildfire smoke plume increased from less than 5% in samples collected close to the emission source to greater than 40% after 3 hours of aging, with little change in downwind TB diameters. The TB mass fraction increased from 2% near the fire to 23±9% downwind. Single-scatter albedo determined from scattering and absorption measurements increased slightly with downwind distance. Mie calculations show this observation is consistent with weak light absorbance by TBs (m=1.56 - 0.02i) but not consistent with order-of-magnitude stronger absorption observed in different settings. The field-derived TB mass fractions reported here indicate that this particle type should be accounted for in biomass-burn emission inventories.

  6. Trans-Pacific transport of dust aerosols from East Asia: Insights gained from multiple observations and modeling.

    PubMed

    Guo, Jianping; Lou, Mengyun; Miao, Yucong; Wang, Yuan; Zeng, Zhaoliang; Liu, Huan; He, Jing; Xu, Hui; Wang, Fu; Min, Min; Zhai, Panmao

    2017-11-01

    East Asia is one of the world's largest sources of dust and anthropogenic pollution. Dust particles originating from East Asia have been recognized to travel across the Pacific to North America and beyond, thereby affecting the radiation incident on the surface as well as clouds aloft in the atmosphere. In this study, integrated analyses are performed focusing on one trans-Pacific dust episode during 12-22 March 2015, based on space-borne, ground-based observations, reanalysis data combined with Hybrid Single Particle Lagrangian Integrated Trajectory Model (HYSPLIT), and the Weather Research and Forecasting Model coupled with Chemistry (WRF-Chem). From the perspective of synoptic patterns, the location and strength of Aleutian low pressure system largely determined the eastward transport of dust plumes towards western North America. Multi-sensor satellite observations reveal that dust aerosols in this episode originated from the Taklimakan and Gobi Deserts. Moreover, the satellite observations suggest that the dust particles can be transformed to polluted particles over the East Asian regions after encountering high concentration of anthropogenic pollutants. In terms of the vertical distribution of polluted dust particles, at the very beginning, they were mainly located in the altitudes ranging from 1 km to 7 km over the source region, then ascended to 2 km-9 km over the Pacific Ocean. The simulations confirm that these elevated dust particles in the lower free troposphere were largely transported along the prevailing westerly jet stream. Overall, observations and modeling demonstrate how a typical springtime dust episode develops and how the dust particles travel over the North Pacific Ocean all the way to North America. Copyright © 2017 Elsevier Ltd. All rights reserved.

  7. A climatology of fine absorbing biomass burning, urban and industrial aerosols detected from satellites

    NASA Astrophysics Data System (ADS)

    Kalaitzi, Nikoleta; Hatzianastassiou, Nikos; Gkikas, Antonis; Papadimas, Christos D.; Torres, Omar; Mihalopoulos, Nikos

    2017-04-01

    Natural biomass burning (BB) along with anthropogenic urban and industrial aerosol particles, altogether labeled here as BU aerosols, contain black and brown carbon which both absorb strongly the solar radiation. Thus, BU aerosols warm significantly the atmosphere also causing adjustments to cloud properties, which traditionally are known as cloud indirect and semi-direct effects. Given the role of the effects of BU aerosols for contemporary and future climate change, and the uncertainty associated with BU, both ascertained by the latest IPCC reports, there is an urgent need for improving our knowledge on the spatial and temporal variability of BU aerosols all over the globe. Over the last few decades, thanks to the rapid development of satellite observational techniques and retrieval algorithms it is now possible to detect BU aerosols based on satellite measurements. However, care must be taken in order to ensure the ability to distinguish BU from other aerosol types usually co-existing in the Earth's atmosphere. In the present study, an algorithm is presented, based on a synergy of different satellite measurements, aiming to identify and quantify BU aerosols over the entire globe and during multiple years. The objective is to build a satellite-based climatology of BU aerosols intended for use for various purposes. The produced regime, namely the spatial and temporal variability of BU aerosols, emphasizes the BU frequency of occurrence and their intensity, in terms of aerosol optical depth (AOD). The algorithm is using the following aerosol optical properties describing the size and atmospheric loading of BU aerosols: (i) spectral AOD, (ii) Ångström Exponent (AE), (iii) Fine Fraction (FF) and (iv) Aerosol Index (AI). The relevant data are taken from Collection 006 MODIS-Aqua, except for AI which is taken from OMI-Aura. The identification of BU aerosols by the algorithm is based on a specific thresholding technique, with AI≥1.5, AE≥1.2 and FF≥0.6 threshold

  8. An Accurate Analytic Approximation for Light Scattering by Non-absorbing Spherical Aerosol Particles

    NASA Astrophysics Data System (ADS)

    Lewis, E. R.

    2017-12-01

    The scattering of light by particles in the atmosphere is a ubiquitous and important phenomenon, with applications to numerous fields of science and technology. The problem of scattering of electromagnetic radiation by a uniform spherical particle can be solved by the method of Mie and Debye as a series of terms depending on the size parameter, x=2πr/λ, and the complex index of refraction, m. However, this solution does not provide insight into the dependence of the scattering on the radius of the particle, the wavelength, or the index of refraction, or how the scattering varies with relative humidity. Van de Hulst demonstrated that the scattering efficiency (the scattering cross section divided by the geometric cross section) of a non-absorbing sphere, over a wide range of particle sizes of atmospheric importance, depends not on x and m separately, but on the quantity 2x(m-1); this is the basis for the anomalous diffraction approximation. Here an analytic approximation for the scattering efficiency of a non-absorbing spherical particle is presented in terms of this new quantity that is accurate over a wide range of particle sizes of atmospheric importance and which readily displays the dependences of the scattering efficiency on particle radius, index of refraction, and wavelength. For an aerosol for which the particle size distribution is parameterized as a gamma function, this approximation also yields analytical results for the scattering coefficient and for the Ångström exponent, with the dependences of scattering properties on wavelength and index of refraction clearly displayed. This approximation provides insight into the dependence of light scattering properties on factors such as relative humidity, readily enables conversion of scattering from one index of refraction to another, and demonstrates the conditions under which the aerosol index (the product of the aerosol optical depth and the Ångström exponent) is a useful proxy for the number of cloud

  9. WRF-Chem Model Simulations of Arizona Dust Storms

    NASA Astrophysics Data System (ADS)

    Mohebbi, A.; Chang, H. I.; Hondula, D.

    2017-12-01

    The online Weather Research and Forecasting model with coupled chemistry module (WRF-Chem) is applied to simulate the transport, deposition and emission of the dust aerosols in an intense dust outbreak event that took place on July 5th, 2011 over Arizona. Goddard Chemistry Aerosol Radiation and Transport (GOCART), Air Force Weather Agency (AFWA), and University of Cologne (UoC) parameterization schemes for dust emission were evaluated. The model was found to simulate well the synoptic meteorological conditions also widely documented in previous studies. The chemistry module performance in reproducing the atmospheric desert dust load was evaluated using the horizontal field of the Aerosol Optical Depth (AOD) from Moderate Resolution Imaging Spectro (MODIS) radiometer Terra/Aqua and Aerosol Robotic Network (AERONET) satellites employing standard Dark Target (DT) and Deep Blue (DB) algorithms. To assess the temporal variability of the dust storm, Particulate Matter mass concentration data (PM10 and PM2.5) from Arizona Department of Environmental Quality (AZDEQ) ground-based air quality stations were used. The promising performance of WRF-Chem indicate that the model is capable of simulating the right timing and loading of a dust event in the planetary-boundary-layer (PBL) which can be used to forecast approaching severe dust events and to communicate an effective early warning.

  10. Aerosol optical properties and direct radiative forcing based on measurements from the China Aerosol Remote Sensing Network (CARSNET) in eastern China

    NASA Astrophysics Data System (ADS)

    Che, Huizheng; Qi, Bing; Zhao, Hujia; Xia, Xiangao; Eck, Thomas F.; Goloub, Philippe; Dubovik, Oleg; Estelles, Victor; Cuevas-Agulló, Emilio; Blarel, Luc; Wu, Yunfei; Zhu, Jun; Du, Rongguang; Wang, Yaqiang; Wang, Hong; Gui, Ke; Yu, Jie; Zheng, Yu; Sun, Tianze; Chen, Quanliang; Shi, Guangyu; Zhang, Xiaoye

    2018-01-01

    Aerosol pollution in eastern China is an unfortunate consequence of the region's rapid economic and industrial growth. Here, sun photometer measurements from seven sites in the Yangtze River Delta (YRD) from 2011 to 2015 were used to characterize the climatology of aerosol microphysical and optical properties, calculate direct aerosol radiative forcing (DARF) and classify the aerosols based on size and absorption. Bimodal size distributions were found throughout the year, but larger volumes and effective radii of fine-mode particles occurred in June and September due to hygroscopic growth and/or cloud processing. Increases in the fine-mode particles in June and September caused AOD440 nm > 1.00 at most sites, and annual mean AOD440 nm values of 0.71-0.76 were found at the urban sites and 0.68 at the rural site. Unlike northern China, the AOD440 nm was lower in July and August (˜ 0.40-0.60) than in January and February (0.71-0.89) due to particle dispersion associated with subtropical anticyclones in summer. Low volumes and large bandwidths of both fine-mode and coarse-mode aerosol size distributions occurred in July and August because of biomass burning. Single-scattering albedos at 440 nm (SSA440 nm) from 0.91 to 0.94 indicated particles with relatively strong to moderate absorption. Strongly absorbing particles from biomass burning with a significant SSA wavelength dependence were found in July and August at most sites, while coarse particles in March to May were mineral dust. Absorbing aerosols were distributed more or less homogeneously throughout the region with absorption aerosol optical depths at 440 nm ˜ 0.04-0.06, but inter-site differences in the absorption Angström exponent indicate a degree of spatial heterogeneity in particle composition. The annual mean DARF was -93 ± 44 to -79 ± 39 W m-2 at the Earth's surface and ˜ -40 W m-2 at the top of the atmosphere (for the solar zenith angle range of 50 to 80°) under cloud-free conditions. The fine mode

  11. An overview of mineral dust modeling over East Asia

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Chen, Siyu; Huang, Jianping; Qian, Yun

    Dust aerosol, one of the most abundant aerosol species in the atmosphere, has significant impacts on the energy balance and climatic feedback of the Earth system through its influence on solar and terrestrial radiation as well as clouds. East Asia is the one of prominent regions of dust generation. The East Asia dust life cycle and associated radiative and climatic effects are the outstanding science issues in understanding climate change at regional and even global scale. In the past decades, numerous dust models have been developed and applied to comprehend a series of dust-related processes studies, including emission, transport, andmore » deposition, and to understand the effects of dust aerosol on the radiation and climate over East Asian. In this paper, we review the recent achievements and progresses in East Asian dust modeling research and discuss the potential challenges in future studies.« less

  12. An anomalous African dust event and its impact on aerosol radiative forcing on the Southwest Atlantic coast of Europe in February 2016.

    PubMed

    Sorribas, M; Adame, J A; Andrews, E; Yela, M

    2017-04-01

    A desert dust (DD) event that had its origin in North Africa occurred on the 20th-23rd of February 2016. The dust transport phenomenon was exceptional because of its unusual intensity during the coldest season. A historical dataset (2006-2015) of February meteorological scenarios using ECMWF fields, meteorological parameters, aerosol optical properties, surface O 3 and AOD retrieved from MODIS at the El Arenosillo observatory (southwestern Spain) were analysed and compared with the levels during the DD event to highlight its exceptionality. Associated with a low-pressure system in western North Africa, flows transported air from the Sahel to Algeria and consequently increased temperatures from the surface to 700hPa by up to 7-9°C relative to the last decade. These conditions favoured the formation of a Saharan air layer. Dust was transported to the north and reached the Western Mediterranean Basin and the Iberian Peninsula. The arrival of the DD event at El Arenosillo did not affect the surface weather conditions or ozone but did impact the aerosol radiative forcing at the top of atmosphere (RF TOA ). Aerosol radiative properties did not change relative to historical; however, the particle size and the amount of the aerosol were significantly higher. The DD event caused an increase (in absolute terms) of the mean aerosol RF TOA to a value of -8.1Wm -2 (long-term climatological value ~-1.5Wm -2 ). The aerosol RF TOA was not very large relative other DD episodes; however, our analysis of the historical data concluded that the importance of this DD event lay in the month of occurrence. European phenological datasets related to extreme atmospheric events predominantly reflect changes that are probably associated with climate change. This work is an example of this phenomenon, showing an event that occurred in a hotspot, the Saharan desert, and its impact two thousand km away. Copyright © 2017 Elsevier B.V. All rights reserved.

  13. Analysis of aerosol composition data for western United States wildfires between 2005 and 2015: Dust emissions, chloride depletion, and most enhanced aerosol constituents.

    PubMed

    Schlosser, Joseph S; Braun, Rachel A; Bradley, Trevor; Dadashazar, Hossein; MacDonald, Alexander B; Aldhaif, Abdulmonam A; Aghdam, Mojtaba Azadi; Mardi, Ali Hossein; Xian, Peng; Sorooshian, Armin

    2017-08-27

    This study examines major wildfires in the western United States between 2005 and 2015 to determine which species exhibit the highest percent change in mass concentration on day of peak fire influence relative to preceding nonfire days. Forty-one fires were examined using the Environmental Protection Agency (EPA) Interagency Monitoring of Protected Visual Environments (IMPROVE) data set. Organic carbon (OC) and elemental carbon (EC) constituents exhibited the highest percent change increase. The sharpest enhancements were for the volatile (OC1) and semivolatile (OC2) OC fractions, suggestive of secondary organic aerosol formation during plume transport. Of the noncarbonaceous constituents, Cl, P, K, NO 3 - , and Zn levels exhibited the highest percent change. Dust was significantly enhanced in wildfire plumes, based on significant enhancements in fine soil components (i.e., Si, Ca, Al, Fe, and Ti) and PM coarse (i.e., PM 10 -PM 2.5 ). A case study emphasized how transport of wildfire plumes significantly impacted downwind states, with higher levels of fine soil and PM coarse at the downwind state (Arizona) as compared to the source of the fires (California). A global model (Navy Aerosol Analysis and Prediction System, NAAPS) did not capture the dust influence over California or Arizona during this case event because it is not designed to resolve dust dynamics in fires, which motivates improved treatment of such processes. Significant chloride depletion was observed on the peak EC day for almost a half of the fires examined. Size-resolved measurements during two specific fires at a coastal California site revealed significant chloride reductions for particle aerodynamic diameters between 1 and 10 μm.

  14. Analysis of aerosol composition data for western United States wildfires between 2005 and 2015: Dust emissions, chloride depletion, and most enhanced aerosol constituents

    NASA Astrophysics Data System (ADS)

    Schlosser, Joseph S.; Braun, Rachel A.; Bradley, Trevor; Dadashazar, Hossein; MacDonald, Alexander B.; Aldhaif, Abdulmonam A.; Aghdam, Mojtaba Azadi; Mardi, Ali Hossein; Xian, Peng; Sorooshian, Armin

    2017-08-01

    This study examines major wildfires in the western United States between 2005 and 2015 to determine which species exhibit the highest percent change in mass concentration on day of peak fire influence relative to preceding nonfire days. Forty-one fires were examined using the Environmental Protection Agency (EPA) Interagency Monitoring of Protected Visual Environments (IMPROVE) data set. Organic carbon (OC) and elemental carbon (EC) constituents exhibited the highest percent change increase. The sharpest enhancements were for the volatile (OC1) and semivolatile (OC2) OC fractions, suggestive of secondary organic aerosol formation during plume transport. Of the noncarbonaceous constituents, Cl, P, K, NO3-, and Zn levels exhibited the highest percent change. Dust was significantly enhanced in wildfire plumes, based on significant enhancements in fine soil components (i.e., Si, Ca, Al, Fe, and Ti) and PMcoarse (i.e., PM10-PM2.5). A case study emphasized how transport of wildfire plumes significantly impacted downwind states, with higher levels of fine soil and PMcoarse at the downwind state (Arizona) as compared to the source of the fires (California). A global model (Navy Aerosol Analysis and Prediction System, NAAPS) did not capture the dust influence over California or Arizona during this case event because it is not designed to resolve dust dynamics in fires, which motivates improved treatment of such processes. Significant chloride depletion was observed on the peak EC day for almost a half of the fires examined. Size-resolved measurements during two specific fires at a coastal California site revealed significant chloride reductions for particle aerodynamic diameters between 1 and 10 μm.

  15. Analysis of aerosol composition data for western United States wildfires between 2005 and 2015: Dust emissions, chloride depletion, and most enhanced aerosol constituents

    PubMed Central

    Schlosser, Joseph S.; Braun, Rachel A.; Bradley, Trevor; Dadashazar, Hossein; MacDonald, Alexander B.; Aldhaif, Abdulmonam A.; Aghdam, Mojtaba Azadi; Mardi, Ali Hossein; Xian, Peng; Sorooshian, Armin

    2017-01-01

    This study examines major wildfires in the western United States between 2005 and 2015 to determine which species exhibit the highest percent change in mass concentration on day of peak fire influence relative to preceding nonfire days. Forty-one fires were examined using the Environmental Protection Agency (EPA) Interagency Monitoring of Protected Visual Environments (IMPROVE) data set. Organic carbon (OC) and elemental carbon (EC) constituents exhibited the highest percent change increase. The sharpest enhancements were for the volatile (OC1) and semivolatile (OC2) OC fractions, suggestive of secondary organic aerosol formation during plume transport. Of the noncarbonaceous constituents, Cl, P, K, NO3−, and Zn levels exhibited the highest percent change. Dust was significantly enhanced in wildfire plumes, based on significant enhancements in fine soil components (i.e., Si, Ca, Al, Fe, and Ti) and PMcoarse (i.e., PM10–PM2.5). A case study emphasized how transport of wildfire plumes significantly impacted downwind states, with higher levels of fine soil and PMcoarse at the downwind state (Arizona) as compared to the source of the fires (California). A global model (Navy Aerosol Analysis and Prediction System, NAAPS) did not capture the dust influence over California or Arizona during this case event because it is not designed to resolve dust dynamics in fires, which motivates improved treatment of such processes. Significant chloride depletion was observed on the peak EC day for almost a half of the fires examined. Size-resolved measurements during two specific fires at a coastal California site revealed significant chloride reductions for particle aerodynamic diameters between 1 and 10 μm. PMID:28955601

  16. Analysis of Light Absorbing Aerosols in Northern Pakistan: Concentration on Snow/Ice, their Source Regions and Impacts on Snow Albedo

    NASA Astrophysics Data System (ADS)

    Gul, C.; Praveen, P. S.; Shichang, K.; Adhikary, B.; Zhang, Y.; Ali, S.

    2016-12-01

    Elemental carbon (EC) and light absorbing organic carbon (OC) are important particulate impurities in snow and ice which significantly reduce the albedo of glaciers and accelerate their melting. Snow and ice samples were collected from Karakorum-Himalayan region of North Pakistan during the summer campaign (May-Jun) 2015 and only snow samples were collected during winter (Dec 2015- Jan 2016). Total 41 surface snow/ice samples were collected during summer campaign along different elevation ranges (2569 to 3895 a.m.s.l) from six glaciers: Sachin, Henarche, Barpu, Mear, Gulkin and Passu. Similarly 18 snow samples were collected from Sust, Hoper, Tawas, Astore, Shangla, and Kalam regions during the winter campaign. Quartz filters were used for filtering of melted snow and ice samples which were then analyzed by thermal optical reflectance (TOR) method to determine the concentration of EC and OC. The average concentration of EC (ng/g), OC (ng/g) and dust (ppm) were found as follows: Passu (249.5, 536.8, 475), Barpu (1190, 397.6, 1288), Gulkin (412, 793, 761), Sachin (911, 2130, 358), Mear (678, 2067, 83) and Henarche (755, 1868, 241) respectively during summer campaign. Similarly, average concentration of EC (ng/g), OC (ng/g) and dust (ppm) was found in the samples of Sust (2506, 1039, 131), Hoper (646, 1153, 76), Tawas (650, 1320, 16), Astore (1305, 2161, 97), Shangla (739, 2079, 31) and Kalam (107, 347, 5) respectively during winter campaign. Two methods were adopted to identify the source regions: one coupled emissions inventory with back trajectories, second with a simple region tagged chemical transport modeling analysis. In addition, CALIPSO subtype aerosol composition indicated that frequency of smoke in the atmosphere over the region was highest followed by dust and then polluted dust. SNICAR model was used to estimate the snow albedo reduction from our in-situ measurements. Snow albedo reduction was observed to be 0.3% to 27.6%. The derived results were used

  17. Simultaneous Retrieval of Effective Refractive Index and Density from Size Distribution and Light Scattering Data: Weakly-Absorbing Aerosol

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kassianov, Evgueni I.; Barnard, James C.; Pekour, Mikhail S.

    2014-10-01

    We propose here a novel approach for retrieving in parallel the effective density and real refractive index of weakly absorbing aerosol from optical and size distribution measurements. Here we define “weakly absorbing” as aerosol single-scattering albedos that exceed 0.95 at 0.5 um.The required optical measurements are the scattering coefficient and the hemispheric backscatter fraction, obtained in this work from an integrating nephelometer. The required size spectra come from a Scanning Mobility Particle Sizer and an Aerodynamic Particle Sizer. The performance of this approach is first evaluated using a sensitivity study with synthetically generated but measurement-related inputs. The sensitivity study revealsmore » that the proposed approach is robust to random noise; additionally the uncertainties of the retrieval are almost linearly proportional to the measurement errors, and these uncertainties are smaller for the real refractive index than for the effective density. Next, actual measurements are used to evaluate our approach. These measurements include the optical, microphysical, and chemical properties of weakly absorbing aerosol which are representative of a variety of coastal summertime conditions observed during the Two-Column Aerosol Project (TCAP; http://campaign.arm.gov/tcap/). The evaluation includes calculating the root mean square error (RMSE) between the aerosol characteristics retrieved by our approach, and the same quantities calculated using the conventional volume mixing rule for chemical constituents. For dry conditions (defined in this work as relative humidity less than 55%) and sub-micron particles, a very good (RMSE~3%) and reasonable (RMSE~28%) agreement is obtained for the retrieved real refractive index (1.49±0.02) and effective density (1.68±0.21), respectively. Our approach permits discrimination between the retrieved aerosol characteristics of sub-micron and sub-10micron particles. The evaluation results also reveal that the

  18. Recent increase in aerosol loading over the Australian arid zone

    NASA Astrophysics Data System (ADS)

    Mitchell, R. M.; Campbell, S. K.; Qin, Y.

    2009-10-01

    Collocated sun photometer and nephelometer measurements at Tinga Tingana in the Australian Outback over the decade 1997-2007 show a significant increase in aerosol loading following the onset of severe drought conditions in 2002. The mean mid-visible scattering coefficient obtained from nephelometer measurements over the period 2003-2007 is approximately double that recorded over the preceding 5 yr, with consistent trends in the column aerosol optical depth derived from the sun photometer. This increase is confined to the season of dust activity, particularly September to March. In contrast, background aerosol levels during May, June and July remained stable. The enhanced aerosol loadings during the latter 5 yr of the study period can be understood as a combination of dune destabilisation through loss of ephemeral vegetation and surface crust, and the changing supply of fluvial sediments to ephemeral lakes and floodplains within the Lake Eyre Basin. Major dust outbreaks are generally highly localised, although significant dust activity was observed at Tinga Tingana on 50% of days when a major event occurred elsewhere in the Lake Eyre Basin, suggesting frequent basin-wide dust mobilisation. Combined analysis of aerosol optical depth and scattering coefficient shows weak correlation between the surface and column aerosol (R2=0.24). The aerosol scale height is broadly distributed with a mode typically between 2-3 km, with clearly defined seasonal variation. Climatological analysis reveals bimodal structure in the annual cycle of aerosol optical depth, with a summer peak related to maximal dust activity, and a spring peak related to lofted fine-mode aerosol. There is evidence for an increase in near-surface aerosol during the period 2003-2007 relative to 1997-2002, consistent with an increase in dust activity. This accords with an independent finding of increasing aerosol loading over the Australian region as a whole, suggesting that rising dust activity over the Lake

  19. Metals and dust in the neutral ISM: the Galaxy, Magellanic Clouds, and damped Lyman-α absorbers

    NASA Astrophysics Data System (ADS)

    De Cia, Annalisa

    2018-05-01

    Context. The presence of dust in the neutral interstellar medium (ISM) dramatically changes the metal abundances that we measure. Understanding the metal content in the neutral ISM, and a direct comparison between different environments, has been hampered to date because of the degeneracy to the observed ISM abundances caused by the effects of metallicity, the presence of dust, and nucleosynthesis. Aims: We study the metal and dust content in the neutral ISM consistently in different environments, and assess the universality of recently discovered sequences of relative abundances. We also intend to assess the validity of [Zn/Fe] as a tracer of dust in the ISM. This has recently been cast into doubt based on observations of stellar abundances, and needs to be addressed before we can safely use it to study the ISM. Methods: In this letter we present a simple comparison of relative abundances observed in the neutral ISM in the Galaxy, the Magellanic Clouds, and damped Lyman-α absorbers (DLAs). The main novelty in this comparison is the inclusion of the Magellanic Clouds. Results: The same sequences of relative abundances are valid for the Galaxy, Magellanic Clouds, and DLAs. These sequences are driven by the presence of dust in the ISM and seem "universal". Conclusions: The metal and dust properties in the neutral ISM appear to follow a similar behaviour in different environments. This suggests that a dominant fraction of the dust budget is built up from grain growth in the ISM depending of the physical conditions and regardless of the star formation history of the system. In addition, the DLA gas behaves like the neutral ISM, at least from a chemical point of view. Finally, despite the deviations in [Zn/Fe] observed in stellar abundances, [Zn/Fe] is a robust dust tracer in the ISM of different environments, from the Galaxy to DLAs.

  20. A parallel direct numerical simulation of dust particles in a turbulent flow

    NASA Astrophysics Data System (ADS)

    Nguyen, H. V.; Yokota, R.; Stenchikov, G.; Kocurek, G.

    2012-04-01

    Due to their effects on radiation transport, aerosols play an important role in the global climate. Mineral dust aerosol is a predominant natural aerosol in the desert and semi-desert regions of the Middle East and North Africa (MENA). The Arabian Peninsula is one of the three predominant source regions on the planet "exporting" dust to almost the entire world. Mineral dust aerosols make up about 50% of the tropospheric aerosol mass and therefore produces a significant impact on the Earth's climate and the atmospheric environment, especially in the MENA region that is characterized by frequent dust storms and large aerosol generation. Understanding the mechanisms of dust emission, transport and deposition is therefore essential for correctly representing dust in numerical climate prediction. In this study we present results of numerical simulations of dust particles in a turbulent flow to study the interaction between dust and the atmosphere. Homogenous and passive dust particles in the boundary layers are entrained and advected under the influence of a turbulent flow. Currently no interactions between particles are included. Turbulence is resolved through direct numerical simulation using a parallel incompressible Navier-Stokes flow solver. Model output provides information on particle trajectories, turbulent transport of dust and effects of gravity on dust motion, which will be used to compare with the wind tunnel experiments at University of Texas at Austin. Results of testing of parallel efficiency and scalability is provided. Future versions of the model will include air-particle momentum exchanges, varying particle sizes and saltation effect. The results will be used for interpreting wind tunnel and field experiments and for improvement of dust generation parameterizations in meteorological models.

  1. Quantification of uncertainty in aerosol optical thickness retrieval arising from aerosol microphysical model and other sources, applied to Ozone Monitoring Instrument (OMI) measurements

    NASA Astrophysics Data System (ADS)

    Määttä, A.; Laine, M.; Tamminen, J.; Veefkind, J. P.

    2014-05-01

    Satellite instruments are nowadays successfully utilised for measuring atmospheric aerosol in many applications as well as in research. Therefore, there is a growing need for rigorous error characterisation of the measurements. Here, we introduce a methodology for quantifying the uncertainty in the retrieval of aerosol optical thickness (AOT). In particular, we concentrate on two aspects: uncertainty due to aerosol microphysical model selection and uncertainty due to imperfect forward modelling. We apply the introduced methodology for aerosol optical thickness retrieval of the Ozone Monitoring Instrument (OMI) on board NASA's Earth Observing System (EOS) Aura satellite, launched in 2004. We apply statistical methodologies that improve the uncertainty estimates of the aerosol optical thickness retrieval by propagating aerosol microphysical model selection and forward model error more realistically. For the microphysical model selection problem, we utilise Bayesian model selection and model averaging methods. Gaussian processes are utilised to characterise the smooth systematic discrepancies between the measured and modelled reflectances (i.e. residuals). The spectral correlation is composed empirically by exploring a set of residuals. The operational OMI multi-wavelength aerosol retrieval algorithm OMAERO is used for cloud-free, over-land pixels of the OMI instrument with the additional Bayesian model selection and model discrepancy techniques introduced here. The method and improved uncertainty characterisation is demonstrated by several examples with different aerosol properties: weakly absorbing aerosols, forest fires over Greece and Russia, and Sahara desert dust. The statistical methodology presented is general; it is not restricted to this particular satellite retrieval application.

  2. Asian dust events of April 1998

    USGS Publications Warehouse

    Husar, R.B.; Tratt, D.M.; Schichtel, B.A.; Falke, S.R.; Li, F.; Jaffe, D.; Gasso, S.; Gill, T.; Laulainen, N.S.; Lu, F.; Reheis, M.C.; Chun, Y.; Westphal, D.; Holben, B.N.; Gueymard, C.; McKendry, I.; Kuring, N.; Feldman, G.C.; McClain, C.; Frouin, R.J.; Merrill, J.; DuBois, D.; Vignola, F.; Murayama, T.; Nickovic, S.; Wilson, W.E.; Sassen, K.; Sugimoto, N.; Malm, W.C.

    2001-01-01

    On April 15 and 19, 1998, two intense dust storms were generated over the Gobi desert by springtime low-pressure systems descending from the northwest. The windblown dust was detected and its evolution followed by its yellow color on SeaWiFS satellite images, routine surface-based monitoring, and through serendipitous observations. The April 15 dust cloud was recirculating, and it was removed by a precipitating weather system over east Asia. The April 19 dust cloud crossed the Pacific Ocean in 5 days, subsided to the surface along the mountain ranges between British Columbia and California, and impacted severely the optical and the concentration environments of the region. In east Asia the dust clouds increased the albedo over the cloudless ocean and land by up to 10-20%, but it reduced the near-UV cloud reflectance, causing a yellow coloration of all surfaces. The yellow colored backscattering by the dust eludes a plausible explanation using simple Mie theory with constant refractive index. Over the West Coast the dust layer has increased the spectrally uniform optical depth to about 0.4, reduced the direct solar radiation by 30-40%, doubled the diffuse radiation, and caused a whitish discoloration of the blue sky. On April 29 the average excess surface-level dust aerosol concentration over the valleys of the West Coast was about 20-50 ??g/m3 with local peaks >100 ??g/m3. The dust mass mean diameter was 2-3 ??m, and the dust chemical fingerprints were evident throughout the West Coast and extended to Minnesota. The April 1998 dust event has impacted the surface aerosol concentration 2-4 times more than any other dust event since 1988. The dust events were observed and interpreted by an ad hoc international web-based virtual community. It would be useful to set up a community-supported web-based infrastructure to monitor the global aerosol pattern for such extreme aerosol events, to alert and to inform the interested communities, and to facilitate collaborative

  3. Validating Above-cloud Aerosol Optical Depth Retrieved from MODIS using NASA Ames Airborne Sun-Tracking Photometric and Spectrometric (AATS and 4STAR) Measurements

    NASA Astrophysics Data System (ADS)

    Jethva, H. T.; Torres, O.; Remer, L. A.; Redemann, J.; Dunagan, S. E.; Livingston, J. M.; Shinozuka, Y.; Kacenelenbogen, M. S.; Segal-Rosenhaimer, M.

    2014-12-01

    Absorbing aerosols produced from biomass burning and dust outbreaks are often found to overlay the lower level cloud decks as evident in the satellite images. In contrast to the cloud-free atmosphere, in which aerosols generally tend to cool the atmosphere, the presence of absorbing aerosols above cloud poses greater potential of exerting positive radiative effects (warming) whose magnitude directly depends on the aerosol loading above cloud, optical properties of clouds and aerosols, and cloud fraction. In recent years, development of algorithms that exploit satellite-based passive measurements of ultraviolet (UV), visible, and polarized light as well as lidar-based active measurements constitute a major breakthrough in the field of remote sensing of aerosols. While the unprecedented quantitative information on aerosol loading above cloud is now available from NASA's A-train sensors, a greater question remains ahead: How to validate the satellite retrievals of above-cloud aerosols (ACA)? Direct measurements of ACA such as carried out by the NASA Ames Airborne Tracking Sunphotometer (AATS) and Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) can be of immense help in validating ACA retrievals. In this study, we validate the ACA optical depth retrieved using the 'color ratio' (CR) method applied to the MODIS cloudy-sky reflectance by using the airborne AATS and 4STAR measurements. A thorough search of the historic AATS-4STAR database collected during different field campaigns revealed five events where biomass burning, dust, and wildfire-emitted aerosols were found to overlay lower level cloud decks observed during SAFARI-2000, ACE-ASIA 2001, and SEAC4RS-2013, respectively. The co-located satellite-airborne measurements revealed a good agreement (root-mean-square-error<0.1 for Aerosol Optical Depth (AOD) at 500 nm) with most matchups falling within the estimated uncertainties in the MODIS retrievals (-10% to +50%). An extensive validation of

  4. On the shape of martian dust and water ice aerosols

    NASA Astrophysics Data System (ADS)

    Pitman, K. M.; Wolff, M. J.; Clancy, R. T.; Clayton, G. C.

    2000-10-01

    Researchers have often calculated radiative properties of Martian aerosols using either Mie theory for homogeneous spheres or semi-empirical theories. Given that these atmospheric particles are randomly oriented, this approach seems fairly reasonable. However, the idea that randomly oriented nonspherical particles have scattering properties equivalent to even a select subset of spheres is demonstratably false} (Bohren and Huffman 1983; Bohren and Koh 1985, Appl. Optics, 24, 1023). Fortunately, recent computational developments now enable us to directly compute scattering properties for nonspherical particles. We have combined a numerical approach for axisymmetric particle shapes, i.e., cylinders, disks, spheroids (Waterman's T-Matrix approach as improved by Mishchenko and collaborators; cf., Mishchenko et al. 1997, JGR, 102, D14, 16,831), with a multiple-scattering radiative transfer algorithm to constrain the shape of water ice and dust aerosols. We utilize a two-stage iterative process. First, we empirically derive a scattering phase function for each aerosol component (starting with some ``guess'') from radiative transfer models of MGS Thermal Emission Spectrometer Emission Phase Function (EPF) sequences (for details on this step, see Clancy et al., DPS 2000). Next, we perform a series of scattering calculations, adjusting our parameters to arrive at a ``best-fit'' theoretical phase function. In this presentation, we provide details on the second step in our analysis, including the derived phase functions (for several characteristic EPF sequences) as well as the particle properties of the best-fit theoretical models. We provide a sensitivity analysis for the EPF model-data comparisons in terms of perturbations in the particle properties (i.e., range of axial ratios, sizes, refractive indices, etc). This work is supported through NASA grant NAGS-9820 (MJW) and JPL contract no. 961471 (RTC).

  5. Tropospheric Aerosols

    NASA Astrophysics Data System (ADS)

    Buseck, P. R.; Schwartz, S. E.

    2003-12-01

    It is widely believed that "On a clear day you can see forever," as proclaimed in the 1965 Broadway musical of the same name. While an admittedly beautiful thought, we all know that this concept is only figurative. Aside from Earth's curvature and Rayleigh scattering by air molecules, aerosols - colloidal suspensions of solid or liquid particles in a gas - limit our vision. Even on the clearest day, there are billions of aerosol particles per cubic meter of air.Atmospheric aerosols are commonly referred to as smoke, dust, haze, and smog, terms that are loosely reflective of their origin and composition. Aerosol particles have arisen naturally for eons from sea spray, volcanic emissions, wind entrainment of mineral dust, wildfires, and gas-to-particle conversion of hydrocarbons from plants and dimethylsulfide from the oceans. However, over the industrial period, the natural background aerosol has been greatly augmented by anthropogenic contributions, i.e., those produced by human activities. One manifestation of this impact is reduced visibility (Figure 1). Thus, perhaps more than in other realms of geochemistry, when considering the composition of the troposphere one must consider the effects of these activities. The atmosphere has become a reservoir for vast quantities of anthropogenic emissions that exert important perturbations on it and on the planetary ecosystem in general. Consequently, much recent research focuses on the effects of human activities on the atmosphere and, through them, on the environment and Earth's climate. For these reasons consideration of the geochemistry of the atmosphere, and of atmospheric aerosols in particular, must include the effects of human activities. (201K)Figure 1. Impairment of visibility by aerosols. Photographs at Yosemite National Park, California, USA. (a) Low aerosol concentration (particulate matter of aerodynamic diameter less than 2.5 μm, PM2.5=0.3 μg m-3; particulate matter of aerodynamic diameter less than 10

  6. Maps of Structured Aerosol Activity During the MY 25 Planet-encircling Dust Storm on Mars

    NASA Astrophysics Data System (ADS)

    Noble, J.; Wilson, R. J.; Cantor, B. A.; Kahre, M. A.; Hollingsworth, J. L.; Bridger, A. F. C.; Haberle, R. M.; Barnes, J.

    2016-12-01

    We have produced a sequence of 42 global maps from Ls=165.1-187.7° that delimit the areal extent of structured aerosol activity based on a synthesis of Mars Global Surveyor (MGS) data, including Mars Orbiter Camera (MOC) daily global maps (DGMs) and wide angle imagery, Thermal Emission Spectrometer (TES) dust and H2O ice opacity, and Mars general circulation model (MGCM) derived dust opacity. The primary motivation of this work is to examine the temporal and spatial relationship between dust storms observed by MOC and baroclinic eddies inferred from Fast Fourier Synoptic Mapping (FFSM) of TES temperatures in order to study the initiation and evolution of Mars year (MY) 25 planet-encircling dust storm (PDS) precursor phase dust storms. A secondary motivation is to provide improved input to MGCM simulations. Assuming that structured dust storms indicate active dust lifting, these maps allow us to define potential dust lifting regions. This work has two implications for martian atmospheric science. First, integration of MGS data has enabled us to develop improved quantitative and qualitative descriptions of storm evolution that may be used to constrain estimates of dust lifting regions, horizontal dust distribution, and to infer associated circulations. Second, we believe that these maps provide better bases and constraints for modeling storm initiation. Based on our analysis of these MGS data, we propose the following working hypothesis to explain the dynamical processes responsible for PDS initiation and expansion. Six eastward-traveling transient baroclinic eddies triggered the MY 25 precursor storms in Hellas during Ls=176.2-184.6° due to the enhanced dust lifting associated with their low-level wind and stress fields. This was followed by a seventh eddy that contributed to expansion on Ls=186.3°. Increased opacity and temperatures from dust lifting associated with the first three eddies enhanced thermal tides which supported further storm initiation and

  7. Utilization of O4 slant column density to derive aerosol layer height from a spaceborne UV-visible hyperspectral sensor: sensitivity and case study

    NASA Astrophysics Data System (ADS)

    Park, S. S.; Kim, J.; Lee, H.; Torres, O.; Lee, K.-M.; Lee, S. D.

    2015-03-01

    The sensitivities of oxygen-dimer (O4) slant column densities (SCDs) to changes in aerosol layer height are investigated using simulated radiances by a radiative transfer model, Linearized Discrete Ordinate Radiative Transfer (LIDORT), and Differential Optical Absorption Spectroscopy (DOAS) technique. The sensitivities of the O4 SCDs to aerosol types and optical properties are also evaluated and compared. Among the O4 absorption bands at 340, 360, 380, and 477 nm, the O4 absorption band at 477 nm is found to be the most suitable to retrieve the aerosol effective height. However, the O4 SCD at 477 nm is significantly influenced not only by the aerosol layer effective height but also by aerosol vertical profiles, optical properties including single scattering albedo (SSA), aerosol optical depth (AOD), and surface albedo. Overall, the error of the retrieved aerosol effective height is estimated to be 414 m (16.5%), 564 m (22.4%), and 1343 m (52.5%) for absorbing, dust, and non-absorbing aerosol, respectively, assuming knowledge on the aerosol vertical distribution type. Using radiance data from the Ozone Monitoring Instrument (OMI), a new algorithm is developed to derive the aerosol effective height over East Asia after the determination of the aerosol type and AOD from the MODerate resolution Imaging Spectroradiometer (MODIS). The retrieved aerosol effective heights are lower by approximately 300 m (27 %) compared to those obtained from the ground-based LIDAR measurements.

  8. Study of physical and sound absorbing property of epoxy blended coir dust biocomposite

    NASA Astrophysics Data System (ADS)

    Nath, G.; Mishra, S. P.

    2016-09-01

    Reinforcement biocomposite has gained more attention recently due to its low cost, abundantly availability, low density, specific properties, easy method of separation, enhanced energy recovery, CO2 neutrality, biodegradability and recyclable in nature. As a waste product of coconut fruit, the coconut coir dust (CCD) obtained from the coconut husk. The biocomposite material prepared from the CCD modified with the proper blended solution with the help of ultrasonic technique. The study of adiabatic compressibility of acetone / water (70/30) worth its blending property for bleaching of CCD. The biocomposite material of CCD was prepared with epoxy resin. The different physical properties such as sound absorption coefficient, thermal conductivity and electrical conductivity were measured. The morphological study of biocomposite and measurement of sound absorption coefficient shows good evidence of sound absorbing characteristics of biocomposite of CCD. The sound absorption property of composite material shows a significant result where as the thermal conductivity and electrical conductivity executes a weak result. Thus biocomposite of CCD can acts as a good sound absorber and band conductor of heat and electric current.

  9. Modeling atmospheric mineral aerosol chemistry to predict heterogeneous photooxidation of SO2

    NASA Astrophysics Data System (ADS)

    Yu, Zechen; Jang, Myoseon; Park, Jiyeon

    2017-08-01

    The photocatalytic ability of airborne mineral dust particles is known to heterogeneously promote SO2 oxidation, but prediction of this phenomenon is not fully taken into account by current models. In this study, the Atmospheric Mineral Aerosol Reaction (AMAR) model was developed to capture the influence of air-suspended mineral dust particles on sulfate formation in various environments. In the model, SO2 oxidation proceeds in three phases including the gas phase, the inorganic-salted aqueous phase (non-dust phase), and the dust phase. Dust chemistry is described as the absorption-desorption kinetics of SO2 and NOx (partitioning between the gas phase and the multilayer coated dust). The reaction of absorbed SO2 on dust particles occurs via two major paths: autoxidation of SO2 in open air and photocatalytic mechanisms under UV light. The kinetic mechanism of autoxidation was first leveraged using controlled indoor chamber data in the presence of Arizona Test Dust (ATD) particles without UV light, and then extended to photochemistry. With UV light, SO2 photooxidation was promoted by surface oxidants (OH radicals) that are generated via the photocatalysis of semiconducting metal oxides (electron-hole theory) of ATD particles. This photocatalytic rate constant was derived from the integration of the combinational product of the dust absorbance spectrum and wave-dependent actinic flux for the full range of wavelengths of the light source. The predicted concentrations of sulfate and nitrate using the AMAR model agreed well with outdoor chamber data that were produced under natural sunlight. For seven consecutive hours of photooxidation of SO2 in an outdoor chamber, dust chemistry at the low NOx level was attributed to 55 % of total sulfate (56 ppb SO2, 290 µg m-3 ATD, and NOx less than 5 ppb). At high NOx ( > 50 ppb of NOx with low hydrocarbons), sulfate formation was also greatly promoted by dust chemistry, but it was suppressed by the competition between NO2 and SO2

  10. The discoloration of the Taj Mahal due to particulate carbon and dust deposition.

    PubMed

    Bergin, M H; Tripathi, S N; Jai Devi, J; Gupta, T; Mckenzie, M; Rana, K S; Shafer, M M; Villalobos, Ana M; Schauer, J J

    2015-01-20

    The white marble domes of the Taj Mahal are iconic images of India that attract millions of visitors every year. Over the past several decades the outer marble surfaces of the Taj Mahal have begun to discolor with time and must be painstakingly cleaned every several years. Although it has been generally believed that the discoloration is in some way linked with poor air quality in the Agra region, the specific components of air pollution responsible have yet to be identified. With this in mind, ambient particulate matter (PM) samples were collected over a one-year period and found to contain relatively high concentrations of light absorbing particles that could potentially discolor the Taj Mahal marble surfaces, that include black carbon (BC), light absorbing organic carbon (brown carbon, BrC), and dust. Analyses of particles deposited to marble surrogate surfaces at the Taj Mahal indicate that a large fraction of the outer Taj Mahal surfaces are covered with particles that contain both carbonaceous components and dust. We have developed a novel approach that estimates the impact of these deposited particles on the visible light surface reflectance, which is in turn used to estimate the perceived color by the human eye. Results indicate that deposited light absorbing dust and carbonaceous particles (both BC and BrC from the combustion of fossil fuels and biomass) are responsible for the surface discoloration of the Taj Mahal. Overall, the results suggest that the deposition of light absorbing particulate matter in regions of high aerosol loading are not only influencing cultural heritage but also the aesthetics of both natural and urban surfaces.

  11. Two chemically distinct light-absorbing pools of urban organic aerosols: A comprehensive multidimensional analysis of trends.

    PubMed

    Paula, Andreia S; Matos, João T V; Duarte, Regina M B O; Duarte, Armando C

    2016-02-01

    The chemical and light-absorption dynamics of organic aerosols (OAs), a master variable in the atmosphere, have yet to be resolved. This study uses a comprehensive multidimensional analysis approach for exploiting simultaneously the compositional changes over a molecular size continuum and associated light-absorption (ultraviolet absorbance and fluorescence) properties of two chemically distinct pools of urban OAs chromophores. Up to 45% of aerosol organic carbon (OC) is soluble in water and consists of a complex mixture of fluorescent and UV-absorbing constituents, with diverse relative abundances, hydrophobic, and molecular weight (Mw) characteristics between warm and cold periods. In contrast, the refractory alkaline-soluble OC pool (up to 18%) is represented along a similar Mw and light-absorption continuum throughout the different seasons. Results suggest that these alkaline-soluble chromophores may actually originate from primary OAs sources in the urban site. This work shows that the comprehensive multidimensional analysis method is a powerful and complementary tool for the characterization of OAs fractions. The great diversity in the chemical composition and optical properties of OAs chromophores, including both water-soluble and alkaline-soluble OC, may be an important contribution to explain the contrasting photo-reactivity and atmospheric behavior of OAs. Copyright © 2015 Elsevier Ltd. All rights reserved.

  12. Combing Visible and Infrared Spectral Tests for Dust Identification

    NASA Technical Reports Server (NTRS)

    Zhou, Yaping; Levy, Robert; Kleidman, Richard; Remer, Lorraine; Mattoo, Shana

    2016-01-01

    The MODIS Dark Target aerosol algorithm over Ocean (DT-O) uses spectral reflectance in the visible, near-IR and SWIR wavelengths to determine aerosol optical depth (AOD) and Angstrom Exponent (AE). Even though DT-O does have "dust-like" models to choose from, dust is not identified a priori before inversion. The "dust-like" models are not true "dust models" as they are spherical and do not have enough absorption at short wavelengths, so retrieved AOD and AE for dusty regions tends to be biased. The inference of "dust" is based on postprocessing criteria for AOD and AE by users. Dust aerosol has known spectral signatures in the near-UV (Deep blue), visible, and thermal infrared (TIR) wavelength regions. Multiple dust detection algorithms have been developed over the years with varying detection capabilities. Here, we test a few of these dust detection algorithms, to determine whether they can be useful to help inform the choices made by the DT-O algorithm. We evaluate the following methods: The multichannel imager (MCI) algorithm uses spectral threshold tests in (0.47, 0.64, 0.86, 1.38, 2.26, 3.9, 11.0, 12.0 micrometer) channels and spatial uniformity test [Zhao et al., 2010]. The NOAA dust aerosol index (DAI) uses spectral contrast in the blue channels (412nm and 440nm) [Ciren and Kundragunta, 2014]. The MCI is already included as tests within the "Wisconsin" (MOD35) Cloud mask algorithm.

  13. The role of cloud contamination, aerosol layer height and aerosol model in the assessment of the OMI near-UV retrievals over the ocean

    NASA Astrophysics Data System (ADS)

    Gassó, Santiago; Torres, Omar

    2016-07-01

    Retrievals of aerosol optical depth (AOD) at 388 nm over the ocean from the Ozone Monitoring Instrument (OMI) two-channel near-UV algorithm (OMAERUV) have been compared with independent AOD measurements. The analysis was carried out over the open ocean (OMI and MODerate-resolution Imaging Spectrometer (MODIS) AOD comparisons) and over coastal and island sites (OMI and AERONET, the AErosol RObotic NETwork). Additionally, a research version of the retrieval algorithm (using MODIS and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) information as constraints) was utilized to evaluate the sensitivity of the retrieval to different assumed aerosol properties. Overall, the comparison resulted in differences (OMI minus independent measurements) within the expected levels of uncertainty for the OMI AOD retrievals (0.1 for AOD < 0.3, 30 % for AOD > 0.3). Using examples from case studies with outliers, the reasons that led to the observed differences were examined with specific purpose to determine whether they are related to instrument limitations (i.e., pixel size, calibration) or algorithm assumptions (such as aerosol shape, aerosol height). The analysis confirms that OMAERUV does an adequate job at rejecting cloudy scenes within the instrument's capabilities. There is a residual cloud contamination in OMI pixels with quality flag 0 (the best conditions for aerosol retrieval according to the algorithm), resulting in a bias towards high AODs in OMAERUV. This bias is more pronounced at low concentrations of absorbing aerosols (AOD 388 nm ˜ < 0.5). For higher aerosol loadings, the bias remains within OMI's AOD uncertainties. In pixels where OMAERUV assigned a dust aerosol model, a fraction of them (< 20 %) had retrieved AODs significantly lower than AERONET and MODIS AODs. In a case study, a detailed examination of the aerosol height from CALIOP and the AODs from MODIS, along with sensitivity tests, was carried out by varying the different assumed parameters in the

  14. The Role of Cloud Contamination, Aerosol Layer Height and Aerosol Model in the Assessment of the OMI Near-UV Retrievals Over the Ocean

    NASA Technical Reports Server (NTRS)

    Gasso, Santiago; Torres, Omar

    2016-01-01

    Retrievals of aerosol optical depth (AOD) at 388 nm over the ocean from the Ozone Monitoring Instrument (OMI) two-channel near-UV algorithm (OMAERUV) have been compared with independent AOD measurements. The analysis was carried out over the open ocean (OMI and MODerate-resolution Imaging Spectrometer (MODIS) AOD comparisons) and over coastal and island sites (OMI and AERONET, the AErosol RObotic NETwork). Additionally, a research version of the retrieval algorithm (using MODIS and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) information as constraints) was utilized to evaluate the sensitivity of the retrieval to different assumed aerosol properties. Overall, the comparison resulted in differences (OMI minus independent measurements) within the expected levels of uncertainty for the OMI AOD retrievals (0.1 for AOD less than 0.3, 30% for AOD greater than 0.3). Using examples from case studies with outliers, the reasons that led to the observed differences were examined with specific purpose to determine whether they are related to instrument limitations (i.e., pixel size, calibration) or algorithm assumptions (such as aerosol shape, aerosol height). The analysis confirms that OMAERUV does an adequate job at rejecting cloudy scenes within the instrument's capabilities. There is a residual cloud contamination in OMI pixels with quality flag 0 (the best conditions for aerosol retrieval according to the algorithm), resulting in a bias towards high AODs in OMAERUV. This bias is more pronounced at low concentrations of absorbing aerosols (AOD 388 nm approximately less than 0.5). For higher aerosol loadings, the bias remains within OMI's AOD uncertainties. In pixels where OMAERUV assigned a dust aerosol model, a fraction of them (less than 20 %) had retrieved AODs significantly lower than AERONET and MODIS AODs. In a case study, a detailed examination of the aerosol height from CALIOP and the AODs from MODIS, along with sensitivity tests, was carried out by

  15. Enhancements to the caliop aerosol subtyping and lidar ratio selection algorithms for level II version 4

    NASA Astrophysics Data System (ADS)

    Omar, A.; Tackett, J.; Kim, M.-H.; Vaughan, M.; Kar, J.; Trepte, C.; Winker, D.

    2018-04-01

    Several enhancements have been implemented for the version 4 aerosol subtyping and lidar ratio selection algorithms of Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP). Version 4 eliminates the confusion between smoke and clean marine aerosols seen in version 3 by modifications to the elevated layer flag definitions used to identify smoke aerosols over the ocean. To differentiate between mixtures of dust and smoke, and dust and marine aerosols, a new aerosol type will be added in the version 4 data products. In the marine boundary layer, moderately depolarizing aerosols are no longer modeled as mixtures of dust and smoke (polluted dust) but rather as mixtures of dust and seasalt (dusty marine). Some lidar ratios have been updated in the version 4 algorithms. In particular, the dust lidar ratios have been adjusted to reflect the latest measurements and model studies.

  16. Characterization of the 3D distribution of ozone and coarse aerosols in the Troposphere using IASI thermal infrared satellite observations

    NASA Astrophysics Data System (ADS)

    Cuesta, J.; Eremenko, M.; Dufour, G.; Hoepfner, M.; Orphal, J.

    2012-04-01

    Both tropospheric ozone and aerosols significantly affect air quality in megacities during pollution events. Moreover, living conditions may be seriously aggravated when such agglomerations are affected by wildfires (e.g. Russian fires over Moscow in 2010), which produce smoke and pollutant precursors, or even during dense desert dust outbreaks (e.g. recurrently over Beijing or Cairo). Moreover, since aerosols diffuse and absorb solar radiation, they have a direct impact on the photochemical production of tropospheric ozone. These interactions during extreme events of high aerosol loads are nowadays poorly known, even though they may significantly affect the tropospheric photochemical equilibrium. In order to address these issues, we have developed a new retrieval technique to jointly characterize the 3D distribution of both tropospheric ozone and coarse aerosols, using spaceborne observations of the infrared spectrometer IASI onboard MetOp-A satellite. Our methodology is based on the inversion of Earth radiance spectra in the atmospheric window from 8 to 12 μm measured by IASI and a «Tikhonov-Philipps»-type regularisation with constraints varying in altitude (as in [Eremenko et al., 2008, GRL; Dufour et al., 2010 ACP]) to simultaneously retrieve ozone profiles, aerosol optical depths at 10 μm and aerosol layer effective heights. Such joint retrieval prevents biases in the ozone profile retrieval during high aerosol load conditions. Aerosol retrievals using thermal infrared radiances mainly account for desert dust and the coarse fraction of biomass burning aerosols. We use radiances from 15 micro-windows within the 8-12 μm atmospheric window, which were carefully chosen (following [Worden et al., 2006 JGR]) for extracting the maximum information on aerosols and ozone and minimizing contamination by other species. We use the radiative transfer code KOPRA, including line-by-line calculations of gas absorption and single scattering for aerosols [Hoepfner et al

  17. Optical Properties of Aeolian Dusts Common to West Texas

    USDA-ARS?s Scientific Manuscript database

    Both recent models and historical events such as the Dust Bowl and volcanic eruptions have illustrated aerosols can play a significant role in climate change through direct and indirect optical effects. Soil dust aerosols generated by Aeolian processes represent a significant fraction of the total ...

  18. Aerosol Radiative Forcing in Asian Continental Outflow

    NASA Technical Reports Server (NTRS)

    Pueschel, R.; Kinne, S.; Redemann, J.; Gore, Warren J. (Technical Monitor)

    2000-01-01

    Aerosols in elevated layers were sampled with FSSP-probes and wire impactors over the Pacific ocean aboard the NASA DC-8 aircraft. Analyses of particle size and morphology identifies two distinctly different aerosol types for cases when the mid-visible extinctions exceed 0.2/km. Smaller sizes (effective radii of 0.2 um) and moderate absorption (mid-visible single scattering albedo of.935) are typical for urban-industrial pollution. Larger sizes (effective radii of 0.7 um) and weak absorption (mid-visible single scattering albedo of 0.985) identify dust. This aerosol classification is in agreement with its origin as determined by airmass back trajectory analysis. Based on lidar vertical profiling, aerosol dominated by dust and urban-industrial pollution above 3km were assigned mid-visible optical depths of 0.50 and 0.27, respectively. Radiative transfer simulations, considering a 50% cloud-cover below the aerosol layers, suggest (on a daily tP C)C> basis) small reductions (-4W/m2) to the energy budget at the top of the atmosphere for both aerosol types. For c' 0 dust, more backscattering of sunlight (weaker solar absorption) is compensated by a stronger greenhouse effect due to larger sizes. Forced reductions to the energy budget at the surface are 12W/m2 for both aerosol types. In contrast, impacts on heating rates within the aerosol layers are quite different: While urban-industrial aerosol warms the layer (at +0.6K/day as solar heating dominates), dust cools (at -0.5K/day as infrared cooling dominates). Sensitivity tests show the dependence of the aerosol climatic impact on the optical depth, particle size, absorptivity, and altitude of the layers, as well as clouds and surface properties. Climatic cooling can be eliminated (1) for the urban-industrial aerosol if absorption is increased to yield a mid-visible single scattering albedo of 0.89, or if the ocean is replaced by a land surface; (2) for the dust aerosol if the effective radius is increased from 0.7 to 1

  19. Predicting the mineral composition of dust aerosols – Part 2: Model evaluation and identification of key processes with observations

    DOE PAGES

    Perlwitz, J. P.; Perez Garcia-Pando, C.; Miller, R. L.

    2015-10-21

    A global compilation of nearly sixty measurement studies is used to evaluate two methods of simulating the mineral composition of dust aerosols in an Earth system model. Both methods are based upon a Mean Mineralogical Table (MMT) that relates the soil mineral fractions to a global atlas of arid soil type. The Soil Mineral Fraction (SMF) method assumes that the aerosol mineral fractions match the fractions of the soil. The MMT is based upon soil measurements after wet sieving, a process that destroys aggregates of soil particles that would have been emitted from the original, undisturbed soil. The second methodmore » approximately reconstructs the emitted aggregates. This model is referred to as the Aerosol Mineral Fraction (AMF) method because the mineral fractions of the aerosols differ from those of the wet-sieved parent soil, partly due to reaggregation. The AMF method remedies some of the deficiencies of the SMF method in comparison to observations. Only the AMF method exhibits phyllosilicate mass at silt sizes, where they are abundant according to observations. In addition, the AMF quartz fraction of silt particles is in better agreement with measured values, in contrast to the overestimated SMF fraction. Measurements at distinct clay and silt particle sizes are shown to be more useful for evaluation of the models, in contrast to the sum over all particles sizes that is susceptible to compensating errors, as illustrated by the SMF experiment. Model errors suggest that allocation of the emitted silt fraction of each mineral into the corresponding transported size categories is an important remaining source of uncertainty. Evaluation of both models and the MMT is hindered by the limited number of size-resolved measurements of mineral content that sparsely sample aerosols from the major dust sources. In conclusion, the importance of climate processes dependent upon aerosol mineral composition shows the need for global and routine mineral measurements.« less

  20. Using the Aerosol Single Scattering Albedo and Angstrom Exponent from AERONET to Determine Aerosol Origins and Mixing States over the Indo-Gangetic Plain

    NASA Astrophysics Data System (ADS)

    Giles, D. M.; Holben, B. N.; Eck, T. F.; Sinyuk, A.; Slutsker, I.; Smirnov, A.; Schafer, J. S.; Dickerson, R. R.; Thompson, A. M.; Tripathi, S. N.; Singh, R. P.; Ghauri, B.

    2012-12-01

    Aerosol mixtures—whether dominated by dust, carbon, sulfates, nitrates, sea salt, or mixtures of them—complicate the retrieval of remotely sensed aerosol properties from satellites and possibly increase the uncertainty of the aerosol radiative impact on climate. Major aerosol source regions in South Asia include the Thar Desert as well as agricultural lands, Himalayan foothills, and large urban centers in and near the Indo-Gangetic Plain (IGP). Over India and Pakistan, seasonal changes in meteorology, including the monsoon (June-September), significantly affect the transport, lifetime, and type of aerosols. Strong monsoonal winds can promote long range transport of dust resulting in mixtures of dust and carbonaceous aerosols, while more stagnant synoptic conditions (e.g., November-January) can prolong the occurrence of urban/industrial pollution, biomass burning smoke, or mixtures of them over the IGP. Aerosol Robotic Network (AERONET) Sun/sky radiometer data are analyzed to show the aerosol optical depth (AOD) seasonality and aerosol dominant mixing states. The Single Scattering Albedo (SSA) and extinction Angstrom exponent (EAE) relationship has been shown to provide sound clustering of dominant aerosol types using long term AERONET site data near known source regions [Giles et al., 2012]. In this study, aerosol type partitioning using the SSA (440 nm) and EAE (440-870 nm) relationship is further developed to quantify the occurrence of Dust, Mixed (e.g., dust and carbonaceous aerosols), Urban/Industrial (U/I) pollution, and Biomass Burning (BB) smoke. Based on EAE thresholds derived from the cluster analysis (for AOD440nm>0.4), preliminary results (2001-2010) for Kanpur, India, show the overall contributions of each dominant particle type (rounded to the nearest 10%): 10% for Dust (EAE≤0.25), 60% for Mixed (0.251.25). In the IGP, BB aerosols may have varying sizes (e.g., corresponding to 1.2

  1. Impacts of absorbing aerosol deposition on snowpack and hydrologic cycle in the Rocky Mountain region based on variable-resolution CESM (VR-CESM) simulations

    NASA Astrophysics Data System (ADS)

    Wu, Chenglai; Liu, Xiaohong; Lin, Zhaohui; Rahimi-Esfarjani, Stefan R.; Lu, Zheng

    2018-01-01

    The deposition of light-absorbing aerosols (LAAs), such as black carbon (BC) and dust, onto snow cover has been suggested to reduce the snow albedo and modulate the snowpack and consequent hydrologic cycle. In this study we use the variable-resolution Community Earth System Model (VR-CESM) with a regionally refined high-resolution (0.125°) grid to quantify the impacts of LAAs in snow in the Rocky Mountain region during the period 1981-2005. We first evaluate the model simulation of LAA concentrations both near the surface and in snow and then investigate the snowpack and runoff changes induced by LAAs in snow. The model simulates similar magnitudes of near-surface atmospheric dust concentrations as observations in the Rocky Mountain region. Although the model underestimates near-surface atmospheric BC concentrations, the model overestimates BC-in-snow concentrations by 35 % on average. The regional mean surface radiative effect (SRE) due to LAAs in snow reaches up to 0.6-1.7 W m-2 in spring, and dust contributes to about 21-42 % of total SRE. Due to positive snow albedo feedbacks induced by the LAA SRE, snow water equivalent is reduced by 2-50 mm and snow cover fraction by 5-20 % in the two regions around the mountains (eastern Snake River Plain and southwestern Wyoming), corresponding to an increase in surface air temperature by 0.9-1.1 °C. During the snow melting period, LAAs accelerate the hydrologic cycle with monthly runoff increases of 0.15-1.00 mm day-1 in April-May and reductions of 0.04-0.18 mm day-1 in June-July in the mountainous regions. Of all the mountainous regions, the Southern Rockies experience the largest reduction of total runoff by 15 % during the later stage of snowmelt (i.e., June and July). Compared to previous studies based on field observations, our estimation of dust-induced SRE is generally 1 order of magnitude smaller in the Southern Rockies, which is ascribed to the omission of larger dust particles (with the diameter > 10 µm) in

  2. Near-Real-Time Detection and Monitoring of Dust Events by Satellite (SeaWIFS, MODIS, and TOMS)

    NASA Technical Reports Server (NTRS)

    Hsu, N. Christina; Tsay, Si-Chee; Herman, Jay R.; Kaufman, Yoram

    2002-01-01

    Over the last few years satellites have given us increasingly detailed information on the size, location, and duration of dust events around the world. These data not only provide valuable feedback to the modelling community as to the fidelity of their aerosol models but are also finding increasing use in near real-time applications. In particular, the ability to locate and track the development of aerosol dust clouds on a near real-time basis is being used by scientists and government to provide warning of air pollution episodes over major urban area. This ability has also become a crucial component of recent coordinated campaigns to study the characteristics of tropospheric aerosols such as dust and their effect on climate. One such recent campaign was ACE-Asia, which was designed to obtain the comprehensive set of ground, aircraft, and satellite data necessary to provide a detailed understanding of atmospheric aerosol particles over the Asian-Pacific region. As part of ACE-Asia, we developed a near real-time data processing and access system to provide satellite data from the polar-orbiting instruments Earth Probe TOMS (in the form of absorbing aerosol index) and SeaWiFS (in the form of aerosol optical thickness, AOT, and Angstrom exponent). The results were available via web access. The location and movement information provided by these data were used both in support of the day-to-day flight planning of ACE-Asia and as input into aerosol transport models. While near real-time SeaWiFS data processing can be performed using either the normal global data product or data obtained via direct broadcast to receiving stations close to the area of interest, near real-time MODIS processing of data to provide aerosol retrievals is currently only available using its direct broadcast capability. In this paper, we will briefly discuss the algorithms used to generate these data. The retrieved aerosol optical thickness and Angstrom exponent from SeaWiFS will be compared with

  3. Multiangle Imaging Spectroradiometer (MISR) Global Aerosol Optical Depth Validation Based on 2 Years of Coincident Aerosol Robotic Network (AERONET) Observations

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.; Gaitley, Barbara J.; Martonchik, John V.; Diner, David J.; Crean, Kathleen A.; Holben, Brent

    2005-01-01

    Performance of the Multiangle Imaging Spectroradiometer (MISR) early postlaunch aerosol optical thickness (AOT) retrieval algorithm is assessed quantitatively over land and ocean by comparison with a 2-year measurement record of globally distributed AERONET Sun photometers. There are sufficient coincident observations to stratify the data set by season and expected aerosol type. In addition to reporting uncertainty envelopes, we identify trends and outliers, and investigate their likely causes, with the aim of refining algorithm performance. Overall, about 2/3 of the MISR-retrieved AOT values fall within [0.05 or 20% x AOT] of Aerosol Robotic Network (AERONET). More than a third are within [0.03 or 10% x AOT]. Correlation coefficients are highest for maritime stations (approx.0.9), and lowest for dusty sites (more than approx.0.7). Retrieved spectral slopes closely match Sun photometer values for Biomass burning and continental aerosol types. Detailed comparisons suggest that adding to the algorithm climatology more absorbing spherical particles, more realistic dust analogs, and a richer selection of multimodal aerosol mixtures would reduce the remaining discrepancies for MISR retrievals over land; in addition, refining instrument low-light-level calibration could reduce or eliminate a small but systematic offset in maritime AOT values. On the basis of cases for which current particle models are representative, a second-generation MISR aerosol retrieval algorithm incorporating these improvements could provide AOT accuracy unprecedented for a spaceborne technique.

  4. Detection of anthropogenic dust using CALIPSO lidar measurements

    NASA Astrophysics Data System (ADS)

    Huang, J. P.; Liu, J. J.; Chen, B.; Nasiri, S. L.

    2015-10-01

    Anthropogenic dusts are those produced by human activities on disturbed soils, which are mainly cropland, pastureland, and urbanized regions, and are a subset of the total dust load which includes natural sources from desert regions. Our knowledge of anthropogenic dusts is still very limited due to a lack of data. To understand the contribution of anthropogenic dust to the total global dust load, it is important to identify it apart from total dust. In this study, a new technique for distinguishing anthropogenic dust from natural dust is proposed by using Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) dust and planetary boundary layer (PBL) height retrievals along with a land use data set. Using this technique, the global distribution of dust is analyzed and the relative contribution of anthropogenic and natural dust sources to regional and global emissions are estimated. Results reveal that local anthropogenic dust aerosol due to human activity, such as agriculture, industrial activity, transportation, and overgrazing, accounts for about 25 % of the global continental dust load. Of these anthropogenic dust aerosols, more than 53 % come from semi-arid and semi-wet regions. Annual mean anthropogenic dust column burden (DCB) values range from 0.42 g m-2, with a maximum in India, to 0.12 g m-2, with a minimum in North America. A better understanding of anthropogenic dust emission will enable us to focus on human activities in these critical regions and with such knowledge we will be more able to improve global dust models and to explore the effects of anthropogenic emission on radiative forcing, climate change, and air quality in the future.

  5. Analysis of aerosol effects on warm clouds over the Yangtze River Delta from multi-sensor satellite observations

    NASA Astrophysics Data System (ADS)

    Liu, Yuqin; de Leeuw, Gerrit; Kerminen, Veli-Matti; Zhang, Jiahua; Zhou, Putian; Nie, Wei; Qi, Ximeng; Hong, Juan; Wang, Yonghong; Ding, Aijun; Guo, Huadong; Krüger, Olaf; Kulmala, Markku; Petäjä, Tuukka

    2017-05-01

    Aerosol effects on low warm clouds over the Yangtze River Delta (YRD, eastern China) are examined using co-located MODIS, CALIOP and CloudSat observations. By taking the vertical locations of aerosol and cloud layers into account, we use simultaneously observed aerosol and cloud data to investigate relationships between cloud properties and the amount of aerosol particles (using aerosol optical depth, AOD, as a proxy). Also, we investigate the impact of aerosol types on the variation of cloud properties with AOD. Finally, we explore how meteorological conditions affect these relationships using ERA-Interim reanalysis data. This study shows that the relation between cloud properties and AOD depends on the aerosol abundance, with a different behaviour for low and high AOD (i.e. AOD < 0.35 and AOD > 0.35). This applies to cloud droplet effective radius (CDR) and cloud fraction (CF), but not to cloud optical thickness (COT) and cloud top pressure (CTP). COT is found to decrease when AOD increases, which may be due to radiative effects and retrieval artefacts caused by absorbing aerosol. Conversely, CTP tends to increase with elevated AOD, indicating that the aerosol is not always prone to expand the vertical extension. It also shows that the COT-CDR and CWP (cloud liquid water path)-CDR relationships are not unique, but affected by atmospheric aerosol loading. Furthermore, separation of cases with either polluted dust or smoke aerosol shows that aerosol-cloud interaction (ACI) is stronger for clouds mixed with smoke aerosol than for clouds mixed with dust, which is ascribed to the higher absorption efficiency of smoke than dust. The variation of cloud properties with AOD is analysed for various relative humidity and boundary layer thermodynamic and dynamic conditions, showing that high relative humidity favours larger cloud droplet particles and increases cloud formation, irrespective of vertical or horizontal level. Stable atmospheric conditions enhance cloud cover

  6. Response of the Water Cycle of West Africa and Atlantic to Radiative Forcing by Saharan Dust

    NASA Technical Reports Server (NTRS)

    Lau, K. M.; Kim, Kyu-Myong; Sud, Yogesh C.; Walker, Gregory L.

    2010-01-01

    The responses of the atmospheric water cycle and climate of West Africa and the Atlantic to radiative forcing of Saharan dust are studied using the NASA finite volume general circulation model (fvGCM), coupled to a mixed layer ocean. We find evidence in support of the "elevated heat pump" (EHP) mechanism that underlines the responses of the atmospheric water cycle to dust forcing as follow. During the boreal summer, as a result of large-scale atmospheric feed back triggered by absorbing dust aerosols, rainfall and cloudiness are enhanced over the West Africa/Easter Atlantic ITCZ, and suppressed over the West Atlantic and Caribbean. region. Shortwave radiation absorption by dust warms the atmosphere and cools the surface, while long wave has the opposite response. The elevated dust layer warms the air over Nest Africa and the eastern Atlantic. The condensation heating associated with the induced deep convection drives and maintains an anomalous large-scale east-west overturning circulation with rising motion over West Africa/eastern Atlantic, and sinking motion over the Caribbean region. The response also includes a strengthening of the West African monsoon, manifested in northward shift of the West Africa precipitation over land, increased low-level westerlies flow over West Africa at the southern edge of the dust layer, and a near surface energy fluxes, resulting in cooling of the Nest African land and the eastern Atlantic, and a warming in the West Atlantic and Caribbean. The EHP effect is most effective for moderate to highly absorbing dusts, and becomes minimized for reflecting dust with single scattering albedo at 0.95 or higher.

  7. An evaluation of the GCA respirable dust monitor 101-1.

    PubMed

    Marple, V A; Rubow, K L

    1978-01-01

    The GCA RDM 101-1 has been evaluated using aerosols of coal, Arizona road dust, silica, potash, and rock (copper ore) particles. The effects of the dust mass concentration, particle size distribution, and dust material on the instrument response were investigated. The instrument was found to measure the mass concentrations of respirable dust aerosols up to about 16 mg/m3 for coal and rock dust and about 20 mg/m3 for silica, potash, and Arizona road dust, providing there is not appreciable mass in the size range below approximateley 0.7 micrometer aerodynamic diameter.

  8. Trans-Pacific transport and evolution of aerosols: Evaluation of quasi-global WRF-Chem simulation with multiple observations

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hu, Zhiyuan; Zhao, Chun; Huang, Jianping

    A fully coupled meteorology-chemistry model (WRF-Chem, the Weather Research and Forecasting model coupled with chemistry) has been configured to conduct quasi-global simulation for 5 years (2010–2014) and evaluated with multiple observation data sets for the first time. The evaluation focuses on the simulation over the trans-Pacific transport region using various reanalysis and observational data sets for meteorological fields and aerosol properties. The simulation generally captures the overall spatial and seasonal variability of satellite retrieved aerosol optical depth (AOD) and absorbing AOD (AAOD) over the Pacific that is determined by the outflow of pollutants and dust and the emissions of marine aerosols.more » The assessment of simulated extinction Ångström exponent (EAE) indicates that the model generally reproduces the variability of aerosol size distributions as seen by satellites. In addition, the vertical profile of aerosol extinction and its seasonality over the Pacific are also well simulated. The difference between the simulation and satellite retrievals can be mainly attributed to model biases in estimating marine aerosol emissions as well as the satellite sampling and retrieval uncertainties. Compared with the surface measurements over the western USA, the model reasonably simulates the observed magnitude and seasonality of dust, sulfate, and nitrate surface concentrations, but significantly underestimates the peak surface concentrations of carbonaceous aerosol likely due to model biases in the spatial and temporal variability of biomass burning emissions and secondary organic aerosol (SOA) production. A sensitivity simulation shows that the trans-Pacific transported dust, sulfate, and nitrate can make significant contribution to surface concentrations over the rural areas of the western USA, while the peaks of carbonaceous aerosol surface concentrations are dominated by the North American emissions. Both the retrievals and simulation show

  9. Trans-Pacific transport and evolution of aerosols: Evaluation of quasi-global WRF-Chem simulation with multiple observations

    DOE PAGES

    Hu, Zhiyuan; Zhao, Chun; Huang, Jianping; ...

    2016-05-10

    A fully coupled meteorology-chemistry model (WRF-Chem, the Weather Research and Forecasting model coupled with chemistry) has been configured to conduct quasi-global simulation for 5 years (2010–2014) and evaluated with multiple observation data sets for the first time. The evaluation focuses on the simulation over the trans-Pacific transport region using various reanalysis and observational data sets for meteorological fields and aerosol properties. The simulation generally captures the overall spatial and seasonal variability of satellite retrieved aerosol optical depth (AOD) and absorbing AOD (AAOD) over the Pacific that is determined by the outflow of pollutants and dust and the emissions of marine aerosols.more » The assessment of simulated extinction Ångström exponent (EAE) indicates that the model generally reproduces the variability of aerosol size distributions as seen by satellites. In addition, the vertical profile of aerosol extinction and its seasonality over the Pacific are also well simulated. The difference between the simulation and satellite retrievals can be mainly attributed to model biases in estimating marine aerosol emissions as well as the satellite sampling and retrieval uncertainties. Compared with the surface measurements over the western USA, the model reasonably simulates the observed magnitude and seasonality of dust, sulfate, and nitrate surface concentrations, but significantly underestimates the peak surface concentrations of carbonaceous aerosol likely due to model biases in the spatial and temporal variability of biomass burning emissions and secondary organic aerosol (SOA) production. A sensitivity simulation shows that the trans-Pacific transported dust, sulfate, and nitrate can make significant contribution to surface concentrations over the rural areas of the western USA, while the peaks of carbonaceous aerosol surface concentrations are dominated by the North American emissions. Both the retrievals and simulation show

  10. Trans-Pacific transport and evolution of aerosols: evaluation of quasi-global WRF-Chem simulation with multiple observations

    NASA Astrophysics Data System (ADS)

    Hu, Zhiyuan; Zhao, Chun; Huang, Jianping; Leung, L. Ruby; Qian, Yun; Yu, Hongbin; Huang, Lei; Kalashnikova, Olga V.

    2016-05-01

    A fully coupled meteorology-chemistry model (WRF-Chem, the Weather Research and Forecasting model coupled with chemistry) has been configured to conduct quasi-global simulation for 5 years (2010-2014) and evaluated with multiple observation data sets for the first time. The evaluation focuses on the simulation over the trans-Pacific transport region using various reanalysis and observational data sets for meteorological fields and aerosol properties. The simulation generally captures the overall spatial and seasonal variability of satellite retrieved aerosol optical depth (AOD) and absorbing AOD (AAOD) over the Pacific that is determined by the outflow of pollutants and dust and the emissions of marine aerosols. The assessment of simulated extinction Ångström exponent (EAE) indicates that the model generally reproduces the variability of aerosol size distributions as seen by satellites. In addition, the vertical profile of aerosol extinction and its seasonality over the Pacific are also well simulated. The difference between the simulation and satellite retrievals can be mainly attributed to model biases in estimating marine aerosol emissions as well as the satellite sampling and retrieval uncertainties. Compared with the surface measurements over the western USA, the model reasonably simulates the observed magnitude and seasonality of dust, sulfate, and nitrate surface concentrations, but significantly underestimates the peak surface concentrations of carbonaceous aerosol likely due to model biases in the spatial and temporal variability of biomass burning emissions and secondary organic aerosol (SOA) production. A sensitivity simulation shows that the trans-Pacific transported dust, sulfate, and nitrate can make significant contribution to surface concentrations over the rural areas of the western USA, while the peaks of carbonaceous aerosol surface concentrations are dominated by the North American emissions. Both the retrievals and simulation show small

  11. Detection of Saharan dust and biomass burning events using near-real-time intensive aerosol optical properties in the north-western Mediterranean

    NASA Astrophysics Data System (ADS)

    Ealo, Marina; Alastuey, Andrés; Ripoll, Anna; Pérez, Noemí; Cruz Minguillón, María; Querol, Xavier; Pandolfi, Marco

    2016-10-01

    The study of Saharan dust events (SDEs) and biomass burning (BB) emissions are both topics of great scientific interest since they are frequent and important polluting scenarios affecting air quality and climate. The main aim of this work is evaluating the feasibility of using near-real-time in situ aerosol optical measurements for the detection of these atmospheric events in the western Mediterranean Basin (WMB). With this aim, intensive aerosol optical properties (SAE: scattering Ångström exponent, AAE: absorption Ångström exponent, SSAAE: single scattering albedo Ångström exponent and g: asymmetry parameter) were derived from multi-wavelength aerosol light scattering, hemispheric backscattering and absorption measurements performed at regional (Montseny; MSY, 720 m a.s.l.) and continental (Montsec; MSA, 1570 m a.s.l.) background sites in the WMB. A sensitivity study aiming at calibrating the measured intensive optical properties for SDEs and BB detection is presented and discussed. The detection of SDEs by means of the SSAAE parameter and Ångström matrix (made up by SAE and AAE) depended on the altitude of the measurement station and on SDE intensity. At MSA (mountain-top site) SSAAE detected around 85 % of SDEs compared with 50 % at the MSY station, where pollution episodes dominated by fine anthropogenic particles frequently masked the effect of mineral dust on optical properties during less intense SDEs. Furthermore, an interesting feature of SSAAE was its capability to detect the presence of mineral dust after the end of SDEs. Thus, resuspension processes driven by summer regional atmospheric circulations and dry conditions after SDEs favoured the accumulation of mineral dust at regional level having important consequences for air quality. On average, SAE, AAE and g ranged between -0.7 and 1, 1.3 and 2.5 and 0.5 and 0.75 respectively during SDEs. Based on the aethalometer model, BB contribution to equivalent black carbon (BC) accounted for 36 and 40

  12. Quantification of model uncertainty in aerosol optical thickness retrieval from Ozone Monitoring Instrument (OMI) measurements

    NASA Astrophysics Data System (ADS)

    Määttä, A.; Laine, M.; Tamminen, J.; Veefkind, J. P.

    2013-09-01

    We study uncertainty quantification in remote sensing of aerosols in the atmosphere with top of the atmosphere reflectance measurements from the nadir-viewing Ozone Monitoring Instrument (OMI). Focus is on the uncertainty in aerosol model selection of pre-calculated aerosol models and on the statistical modelling of the model inadequacies. The aim is to apply statistical methodologies that improve the uncertainty estimates of the aerosol optical thickness (AOT) retrieval by propagating model selection and model error related uncertainties more realistically. We utilise Bayesian model selection and model averaging methods for the model selection problem and use Gaussian processes to model the smooth systematic discrepancies from the modelled to observed reflectance. The systematic model error is learned from an ensemble of operational retrievals. The operational OMI multi-wavelength aerosol retrieval algorithm OMAERO is used for cloud free, over land pixels of the OMI instrument with the additional Bayesian model selection and model discrepancy techniques. The method is demonstrated with four examples with different aerosol properties: weakly absorbing aerosols, forest fires over Greece and Russia, and Sahara dessert dust. The presented statistical methodology is general; it is not restricted to this particular satellite retrieval application.

  13. Effect of tropospheric aerosols upon atmospheric infrared cooling rates

    NASA Technical Reports Server (NTRS)

    Harshvardhan, MR.; Cess, R. D.

    1978-01-01

    The effect of tropospheric aerosols on atmospheric infrared cooling rates is investigated by the use of recent models of infrared gaseous absorption. A radiative model of the atmosphere that incorporates dust as an absorber and scatterer of infrared radiation is constructed by employing the exponential kernel approximation to the radiative transfer equation. Scattering effects are represented in terms of a single scattering albedo and an asymmetry factor. The model is applied to estimate the effect of an aerosol layer made of spherical quartz particles on the infrared cooling rate. Calculations performed for a reference wavelength of 0.55 microns show an increased greenhouse effect, where the net upward flux at the surface is reduced by 10% owing to the strongly enhanced downward emission. There is a substantial increase in the cooling rate near the surface, but the mean cooling rate throughout the lower troposphere was only 10%.

  14. Characterization of Asian Dust Properties Near Source Region During ACE-Asia

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Hsu, N. Christina; King, Michael D.; Kaufman, Yoram J.; Herman, Jay R.

    2004-01-01

    Asian dust typically originates in desert areas far from polluted urban regions. During transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian aerosols is of special importance in regional-to-global climate issues such as radiative forcing, the hydrological cycle, and primary biological productivity in the mid-Pacific Ocean. During ACE-Asia campaign, we have acquired ground- based (temporal) and satellite (spatial) measurements to infer aerosol physical/optical/radiative properties, column precipitable water amount, and surface reflectivity over this region. The inclusion of flux measurements permits the determination of aerosol radiative flux in addition to measurements of loading and optical depth. At the time of the Terra/MODIS, SeaWiFS, TOMS and other satellite overpasses, these ground-based observations can provide valuable data to compare with satellite retrievals over land. In this paper, we will demonstrate new capability of the Deep Blue algorithm to track the evolution of the Asian dust storm from sources to sinks. Although there are large areas often covered by clouds in the dust season in East Asia, this algorithm is able to distinguish heavy dust from clouds over the entire regions. Examination of the retrieved daily maps of dust plumes over East Asia clearly identifies the sources contributing to the dust loading in the atmosphe. We have compared the satellite retrieved aerosol optical thickness to the ground-based measurements and obtained a reasonable agreement between these two. Our results also indicate that there is a large difference in the retrieved value of spectral single scattering albedo of windblown dust between different

  15. Ice nucleation onto Arizona test dust at cirrus temperatures: effect of temperature and aerosol size on onset relative humidity.

    PubMed

    Kanji, Z A; Abbatt, J P D

    2010-01-21

    The University of Toronto Continuous Flow Diffusion Chamber (UT-CFDC) was used to study ice formation onto monodisperse Arizona Test Dust (ATD) particles. The onset relative humidity with respect to ice (RH(i)) was measured as a function of temperature in the range 251-223 K for 100 nm ATD particles. It was found that for 0.1% of the particles to freeze, water saturation was required at all temperatures except 223 K where particles activated at RH(i) below water saturation. At this temperature, where deposition mode freezing is occurring, we find that the larger the particle size, the lower the onset RH(i). We also demonstrate that the total number of particles present may influence the onset RH(i) observed. The surface area for ice activation, aerosol size, and temperature must all be considered when reporting onset values of ice formation onto ATD mineral dust particles. In addition, we calculate nucleation rates and contact angles of ice germs with ATD aerosols which indicate that there exists a range of active sites on the surface with different efficiencies for activating ice formation.

  16. South Asian aerosols in perspective: Preface to the special issue

    NASA Astrophysics Data System (ADS)

    Moorthy, K. Krishna; Satheesh, S. K.; Sarin, M. M.; Panday, Arnico K.

    2016-01-01

    reported that enhanced warming due to atmospheric BC at higher levels is responsible for the faster melting rates of snowfields and of white glaciers (ones that are not debris-covered); some studies have revealed that the snow albedo forcing overwhelms and is more important for older snow (Nair et al., 2013). Evidence on the record of BC and dust deposition in the Himalayan region is only beginning to emerge (Ming et al., 2008), based on ice-core studies. The full implications of deposition of absorbing aerosols (BC, brown carbon (BrC), and dust) on the Himalayan ice-pack and glaciers remain to be understood.

  17. Assessment of State-of-the-Art Dust Emission Scheme in GEOS

    NASA Technical Reports Server (NTRS)

    Darmenov, Anton; Liu, Xiaohong; Prigent, Catherine

    2017-01-01

    The GEOS modeling system has been extended with state of the art parameterization of dust emissions based on the vertical flux formulation described in Kok et al 2014. The new dust scheme was coupled with the GOCART and MAM aerosol models. In the present study we compare dust emissions, aerosol optical depth (AOD) and radiative fluxes from GEOS experiments with the standard and new dust emissions. AOD from the model experiments are also compared with AERONET and satellite based data. Based on this comparative analysis we concluded that the new parameterization improves the GEOS capability to model dust aerosols originating from African sources, however it lead to overestimation of dust emissions from Asian and Arabian sources. Further regional tuning of key parameters controlling the threshold friction velocity may be required in order to achieve more definitive and uniform improvement in the dust modeling skill.

  18. Aerosol impacts on climate and environment over East Asia

    NASA Astrophysics Data System (ADS)

    Nakata, M.; Sano, I.; Mukai, S.

    2014-12-01

    It is well known that the aerosol distribution in East Asia is complex due to both the increasing emissions of the anthropogenic aerosols associated with economic growth and the behavior of natural dusts. Therefore, detailed observations of atmospheric particles in East Asian are important. It is concerned about the change of concentration of aerosols causes various effects on the climate by directly and indirectly modifying the optical properties and lifetimes of cloud. In addition to radiation budget change, aerosol has a significant potential to change cloud and precipitation. These circulation fields change influence on emission of natural aerosols such as dust aerosols and sea salt aerosols. Also, air pollution in megacities in East Asia has become a serious problem. Especially problematic are fine particles called PM2.5, whose diameter is 2.5 mm or less. Particulate matter (PM) pollution as indicated by high PM2.5 readings will cause a spike in the mortality rate of patients suffering from heart and lung diseases. Because fine particles are much smaller than inhalable coarse particles, the can penetrate deeper into the lungs and cause more severe effects on human health. Anthropogenic sources of PM2.5 include automobiles, factories, coal-burning power plants, and heaters in homes. It is well known that the size of dust particles decreases during long-range transport via westerly winds, and the resulting dust storms can contain high concentrations of fine particles. Accordingly, PM2.5 concentrations correspond well to both anthropogenic and dust aerosols. This work intends to investigate impacts of aerosol on regional climate change and environment over East Asia using observations and model simulations.

  19. Radiative impact of a heavy dust storm over India and surrounding oceanic regions

    NASA Astrophysics Data System (ADS)

    Kedia, Sumita; Kumar, Rajesh; Islam, Sahidul; Sathe, Yogesh; Kaginalkar, Akshara

    2018-07-01

    Efficient management of frequently occurring destructive dust storms requires an in-depth understanding of the extent of impacts of such events. Due to limited availability of observational data, it is difficult to understand/estimate the impact of dust aerosols on the Earth's radiation budget in detail. This study, applies a regional model, Weather Research and Forecasting model with chemistry (WRF-Chem), to investigate the impact of an intense dust storm that originated over the Arabian peninsula during 01-02 April 2015 and transported towards the Indian subcontinent by the westerly winds. Two identical numerical experiments are designed, each for 15 days, one with and another without dust aerosols, to estimate the impact of the dust storm over the Indian subcontinent and adjoining regions. WRF-Chem model reproduced the spatial, temporal as well as the vertical distribution of dust plume reasonably well. Model results show significant changes in aerosol optical, physical and radiative properties due to the dominance of coarse mode aerosols in the atmosphere during the dust storm. Analysis of vertical profiles of particulate matter (PM10) concentration reveals the presence of dust aerosols extending from the surface to altitudes as high as 3-4 km during the dust storm period. The dust storm induced a cooling effect at the surface via reduction in shortwave (SW) radiative flux. A substantial decrease in temperature is also seen at 850 hPa due to dust, indicating a significant impact of dust layer on the atmospheric temperature profile. Atmospheric heating due to dust aerosols in the SW region is found to be compensated up to a large extent by longwave (LW) cooling effect of dust. The net dust induced radiative perturbation at the top of the atmosphere (TOA) over different regions is negative and varied from -2.49 to -0.34 Wm-2, while it is in the range of -0.62 to + 0.32 Wm-2 at the surface.

  20. Respiratory health effects and exposure to superabsorbent polymer and paper dust - an epidemiological study

    PubMed Central

    2011-01-01

    Background The primary aim of the present study was to investigate if exposure to dust from absorbent hygiene products containing superabsorbent polymer is related to symptoms from the airways and from the eyes. The secondary aim was to estimate the current exposure to superabsorbent polymer among production and maintenance workers in a plant producing hygiene products. Methods The cohort comprised 1043 workers of whom 689 were exposed to super absorbent polymer and 804 were exposed to paper dust (overlapping groups). There was 186 workers not exposed to either superabsorbent polymer or to paper dust They were investigated with a comprehensive questionnaire about exposure, asthma, rhinitis and symptoms from eyes and airways. The results were analyzed with logistic regression models adjusting for sex, age, atopy and smoking habits. An aerosol sampler equipped with a polytetrafluoroethylene filter with 1 μm pore size was used for personal samplings in order to measure inhalable dust and superabsorbent polymer. Results The prevalence of nasal crusts (OR 1.4, 95% CI 1.01-2.0) and nose-bleeding (OR 1.7, 95% CI 1.2-2.4) was increased among the paper dust exposed workers (adjusted for superabsorbent polymer exposure). There were no significant effects associated with exposure to superabsorbent polymer (adjusted for paper dust exposure). The average exposure to inhalable levels of total dust (paper dust) varied between 0.40 and 1.37 mg/m3. For superabsorbent polymer dust the average exposure varied between 0.02 and 0.81 mg/m3. Conclusions In conclusion, our study shows that workers manufacturing diapers in the hygiene industry have an increased prevalence of symptoms from the nose, especially nose-bleeding. There was no relation between exposure to superabsorbent polymer and symptoms from eyes, nose or respiratory tract, but exposure to paper dust was associated with nose-bleeding and nasal crusts. This group of workers had also a considerable exposure to superabsorbent

  1. Regional Aerosol Forcing over India: Preliminary Results from the South West Asian Aerosol-Monsoon Interactions (SWAAMI) Aircraft Experiment

    NASA Astrophysics Data System (ADS)

    Morgan, W.; Brooks, J.; Fox, C.; Haslett, S.; Liu, D.; Kompalli, S. K.; Pathak, H.; Manoj, M. R.; Allan, J. D.; Haywood, J. M.; Highwood, E.; Langridge, J.; Nanjundaiah, R. S.; Krishnamoorthy, K.; Babu, S. S.; Satheesh, S. K.; Turner, A. G.; Coe, H.

    2016-12-01

    Aerosol particles from multiple sources across the Indian subcontinent build up to form a dense and extensive haze across the region in advance of the monsoon. These aerosols are thought to perturb the regional radiative balance and hydrological cycle, which may have a significant impact on the monsoon circulation, as well as influencing the associated cloud and rainfall of the system. However the nature and magnitude of such impacts are poorly understood or constrained. Major uncertainties relevant to the regional aerosol burden include its vertical distribution, the relative contribution of different pollution sources and natural emissions and the role of absorbing aerosol species (black carbon and mineral dust). The South West Asian Aerosol-Monsoon Interactions (SWAAMI) project sought to address these major uncertainties by conducting an airborne experiment during June/July 2016 on-board the UK Facility for Airborne Atmospheric Measurement (FAAM) BAe-146 research aircraft. Based out of Lucknow in the), The aircraft conducted multiple flights from Lucknow in the heart of the Indo-Gangetic Plain (IGP) in advance of the monsoon and during the onset phase. The spatial and vertical distribution of aerosol was evaluated across northern India, encompassing drier desert-like regions to the west, heavily populated urban and industrial centres over the IGP and air masses in outflow regions to the south-east towards the Bay of Bengal. Principal measurements included aerosol chemical composition using an Aerodyne Aerosol Mass Spectrometer and a DMT Single Particle Soot Photometer, alongside a Leosphere backscatter LIDAR. Sulphate was a major contributor to the aerosol burden across India, while the organic aerosol was elevated and more dominant over the most polluted regions of the IGP. Substantial aerosol concentrations were frequently observed up to altitudes of approximately 6km, with notable changes in aerosol chemical and physical properties when comparing different

  2. Three Dimensional Aerosol Climatology over India and the North Indian Ocean

    NASA Astrophysics Data System (ADS)

    Adams, A.; Zhang, C.

    2013-12-01

    Numerical models are indispensable tools to study aerosol effects on climate, including both aerosol direct and indirect radiative effects and their role in precipitation. But, agreement among the models has not been achieved, and thus it is not possible to accurately and confidently attain estimates of aerosol effects on climate. The lack of reliable knowledge on global three-dimensional (3D) aerosol climatology has prevented us from assessing the degree to which the disagreement in their aerosol climatic effects may come from differences of aerosol vertical structures in their simulations. To that end, we created a six year, global 3D extinction coefficient dataset for each aerosol species identifiable by the Level 2, Version 3, 5 km Aerosol Profile product from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) as a tool to improve 3D model representations. Here we describe the 3D structure of aerosol in the Middle East, India, and the Northern Indian Ocean and some of the interesting dynamical features responsible for the vertical structure and external mixing of aerosol species. One interesting feature in the 3D structure during boreal summer is a well-defined EC core located 0 - 10°N, 40°E - 90°E (Somalia across the Indian subcontinent), centered at 3 km. This is controlled by a shallow meridional circulation about the core. Additionally, the Somali Low-Level Jet exists at this location, but is usually located below the core (~850 mb). Another interesting feature is a strong EC core located 0 - 15°N, 60°E - 90°E below 0.5 km. Polluted dust (external mixture of dust and smoke) and marine aerosol are collocated in this area with maximum AODs of ~0.5 and ~0.2 respectively. Due to the wind stress over ocean, collocation of aerosol species, altitude, and lack of transport pathway for polluted dust, it is possible that this is an example of aerosol misclassification by

  3. Utilization of O4 slant column density to derive aerosol layer height from a space-borne UV-visible hyperspectral sensor: sensitivity and case study

    NASA Astrophysics Data System (ADS)

    Park, Sang Seo; Kim, Jhoon; Lee, Hanlim; Torres, Omar; Lee, Kwang-Mog; Lee, Sang Deok

    2016-02-01

    The sensitivities of oxygen-dimer (O4) slant column densities (SCDs) to changes in aerosol layer height are investigated using the simulated radiances by a radiative transfer model, the linearized pseudo-spherical vector discrete ordinate radiative transfer (VLIDORT), and the differential optical absorption spectroscopy (DOAS) technique. The sensitivities of the O4 index (O4I), which is defined as dividing O4 SCD by 1040 molecules2 cm-5, to aerosol types and optical properties are also evaluated and compared. Among the O4 absorption bands at 340, 360, 380, and 477 nm, the O4 absorption band at 477 nm is found to be the most suitable to retrieve the aerosol effective height. However, the O4I at 477 nm is significantly influenced not only by the aerosol layer effective height but also by aerosol vertical profiles, optical properties including single scattering albedo (SSA), aerosol optical depth (AOD), particle size, and surface albedo. Overall, the error of the retrieved aerosol effective height is estimated to be 1276, 846, and 739 m for dust, non-absorbing, and absorbing aerosol, respectively, assuming knowledge on the aerosol vertical distribution shape. Using radiance data from the Ozone Monitoring Instrument (OMI), a new algorithm is developed to derive the aerosol effective height over East Asia after the determination of the aerosol type and AOD from the MODerate resolution Imaging Spectroradiometer (MODIS). About 80 % of retrieved aerosol effective heights are within the error range of 1 km compared to those obtained from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements on thick aerosol layer cases.

  4. Overview of the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Forcing on the Mediterranean Climate (ChArMEx/ADRIMED) summer 2013 campaign

    NASA Astrophysics Data System (ADS)

    Mallet, M.; Dulac, F.; Formenti, P.; Nabat, P.; Sciare, J.; Roberts, G.; Pelon, J.; Ancellet, G.; Tanré, D.; Parol, F.; di Sarra, A.; Alados, L.; Arndt, J.; Auriol, F.; Blarel, L.; Bourrianne, T.; Brogniez, G.; Chazette, P.; Chevaillier, S.; Claeys, M.; D'Anna, B.; Denjean, C.; Derimian, Y.; Desboeufs, K.; Di Iorio, T.; Doussin, J.-F.; Durand, P.; Féron, A.; Freney, E.; Gaimoz, C.; Goloub, P.; Gómez-Amo, J. L.; Granados-Muñoz, M. J.; Grand, N.; Hamonou, E.; Jankowiak, I.; Jeannot, M.; Léon, J.-F.; Maillé, M.; Mailler, S.; Meloni, D.; Menut, L.; Momboisse, G.; Nicolas, J.; Podvin, J.; Pont, V.; Rea, G.; Renard, J.-B.; Roblou, L.; Schepanski, K.; Schwarzenboeck, A.; Sellegri, K.; Sicard, M.; Solmon, F.; Somot, S.; Torres, B.; Totems, J.; Triquet, S.; Verdier, N.; Verwaerde, C.; Wenger, J.; Zapf, P.

    2015-07-01

    intense biomass burning events in the region. However, numerous mineral dust plumes were observed during the campaign with main sources located in Morocco, Algeria and Tunisia, leading to aerosol optical depth (AOD) values ranging between 0.2 to 0.6 (at 440 nm) over the western and central Mediterranean basins. Associated aerosol extinction values measured on-board the ATR-42 within the dust plume show local maxima reaching up to 150 Mm-1. Non negligible aerosol extinction (about 50 Mm-1) was also been observed within the Marine Boundary Layer (MBL). By combining ATR-42 extinction, absorption and scattering measurements, a complete optical closure has been made revealing excellent agreement with estimated optical properties. Associated calculations of the dust single scattering albedo (SSA) have been conducted, which show a moderate variability (from 0.90 to 1.00 at 530 nm). In parallel, active remote-sensing observations from the surface and onboard the F-20 aircraft suggest a complex vertical structure of particles and distinct aerosol layers with sea-salt and pollution located within the MBL, and mineral dust and/or aged north American smoke particles located above (up to 6-7 km in altitude). Aircraft and balloon-borne observations show particle size distributions characterized by large aerosols (> 10 μm in diameter) within dust plumes. In terms of shortwave (SW) direct forcing, in-situ surface and aircraft observations have been merged and used as inputs in 1-D radiative transfer codes for calculating the direct radiative forcing (DRF). Results show significant surface SW instantaneous forcing (up to -90 W m-2 at noon). Associated 3-D modeling studies from regional climate (RCM) and chemistry transport (CTM) models indicate a relatively good agreement for simulated AOD compared with measurements/observations from the AERONET/PHOTONS network and satellite data, especially for long-range dust transport. Calculations of the 3-D SW (clear-sky) surface DRF indicate an

  5. Aerosol composition and source apportionment in Santiago de Chile

    NASA Astrophysics Data System (ADS)

    Artaxo, Paulo; Oyola, Pedro; Martinez, Roberto

    1999-04-01

    Santiago de Chile, São Paulo and Mexico City are Latin American urban areas that suffer from heavy air pollution. In order to study air pollution in Santiago area, an aerosol source apportionment study was designed to measure ambient aerosol composition and size distribution for two downtown sampling sites in Santiago. The aerosol monitoring stations were operated in Gotuzo and Las Condes during July and August 1996. The study employed stacked filter units (SFU) for aerosol sampling, collecting fine mode aerosol (dp<2 μm) and coarse mode aerosol (2Aerosol mass (PM 10 mass of particles smaller than 10 μm) and black carbon concentration were also measured. Particle-Induced X-ray Emission (PIXE) was used to measure the concentration of 22 trace elements at levels below 0.5 ng m -3. Quantitative aerosol source apportionment was performed using Absolute Principal Factor Analysis (APFA). Very high aerosol concentrations were observed (up to 400 μg/m 3 PM 10). The main aerosol particle sources in Santiago are resuspended soil dust and traffic emissions. Coarse particles account for 63% of PM 10 aerosol in Gotuzo and 53% in Las Condes. A major part of this component is resuspended soil dust. In the fine fraction, resuspended soil dust accounts for 15% of fine mass, and the aerosols associated with transportation activities account for a high 64% of the fine particle mass. Sulfate particle is an important component of the aerosol in Santiago, mainly originating from gas-to-particle conversion from SO 2. In the Gotuzo site, sulfates are the highest aerosol component, accounting for 64.5% of fine mass. Direct traffic emissions are generally mixed with resuspended soil dust. It is difficult to separate the two components, because the soil dust in downtown Santiago is contaminated with Pb, Br, Cl, and other heavy metals that are also tracers for traffic emissions. Residual oil combustion is observed, with the presence of V, S and Ni. An

  6. Far-Reaching Impacts of African Dust- A Calipso Perspective

    NASA Technical Reports Server (NTRS)

    Yu, Hongbin; Chin, Mian; Yuan, Tianle; Bian, Huisheng; Prospero, Joseph; Omar, Ali; Remer, Lorraine; Winker, David; Yang, Yuekui; Zhang, Yan; hide

    2014-01-01

    African dust can transport across the tropical Atlantic and reach the Amazon basin, exerting far-reaching impacts on climate in downwind regions. The transported dust influences the surface-atmosphere interactions and cloud and precipitation processes through perturbing the surface radiative budget and atmospheric radiative heating and acting as cloud condensation nuclei and ice nuclei. Dust also influences biogeochemical cycle and climate through providing nutrients vital to the productivity of ocean biomass and Amazon forests. Assessing these climate impacts relies on an accurate quantification of dust transport and deposition. Currently model simulations show extremely large diversity, which calls for a need of observational constraints. Kaufman et al. (2005) estimated from MODIS aerosol measurements that about 144 Tg of dust is deposited into the tropical Atlantic and 50 Tg of dust into the Amazon in 2001. This estimated dust import to Amazon is a factor of 3-4 higher than other observations and models. However, several studies have argued that the oversimplified characterization of dust vertical profile in the study would have introduced large uncertainty and very likely a high bias. In this study we quantify the trans-Atlantic dust transport and deposition by using 7 years (2007-2013) observations from CALIPSO lidar. CALIPSO acquires high-resolution aerosol extinction and depolarization profiles in both cloud-free and above-cloud conditions. The unique CALIPSO capability of profiling aerosols above clouds offers an unprecedented opportunity of examining uncertainties associated with the use of MODIS clear-sky data. Dust is separated from other types of aerosols using the depolarization measurements. We estimated that on the basis of 7-year average, 118142 Tg of dust is deposited into the tropical Atlantic and 3860 Tg of dust into the Amazon basin. Substantial interannual variations are observed during the period, with the maximum to minimum ratio of about 1

  7. Improvement in Clouds and the Earth's Radiant Energy System/Surface and Atmosphere Radiation Budget Dust Aerosol Properties, Effects on Surface Validation of Clouds and Radiative Swath

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Rutan, D.; Rose, F.; Charlock, T.P.

    2005-03-18

    Within the Clouds and the Earth's Radiant Energy System (CERES) science team (Wielicki et al. 1996), the Surface and Atmospheric Radiation Budget (SARB) group is tasked with calculating vertical profiles of heating rates, globally, and continuously, beneath CERES footprint observations of Top of Atmosphere (TOA) fluxes. This is accomplished using a fast radiative transfer code originally developed by Qiang Fu and Kuo-Nan Liou (Fu and Liou 1993) and subsequently highly modified by the SARB team. Details on the code and its inputs can be found in Kato et al. (2005) and Rose and Charlock (2002). Among the many required inputsmore » is characterization of the vertical column profile of aerosols beneath each footprint. To do this SARB combines aerosol optical depth information from the moderate-resolution imaging spectroradiometer (MODIS) instrument along with aerosol constituents specified by the Model for Atmosphere and Chemical Transport (MATCH) of Collins et al. (2001), and aerosol properties (e.g. single scatter albedo and asymmetry parameter) from Tegen and Lacis (1996) and OPAC (Hess et al. 1998). The publicly available files that include these flux profiles, called the Clouds and Radiative Swath (CRS) data product, available from the Langley Atmospheric Sciences Data Center (http://eosweb.larc.nasa.gov/). As various versions of the code are completed, publishable results are named ''Editions.'' After CRS Edition 2A was finalized it was found that dust aerosols were too absorptive. Dust aerosols have subsequently been modified using a new set of properties developed by Andy Lacis and results have been released in CRS Edition 2B. This paper discusses the effects of changing desert dust aerosol properties, which can be significant for the radiation budget in mid ocean, a few thousand kilometers from the source regions. Resulting changes are validated via comparison of surface observed fluxes from the Saudi Solar Village surface site (Myers et al. 1999), and the E

  8. Imaginary refractive index and other microphysical properties of volcanic ash, Sarahan dust, and other mineral aerosols

    NASA Astrophysics Data System (ADS)

    Rocha Lima, A.; Martins, J.; Krotkov, N. A.; Artaxo, P.; Todd, M.; Ben Ami, Y.; Dolgos, G.; Espinosa, R.

    2013-12-01

    Aerosol properties are essential to support remote sensing measurements, atmospheric circulation and climate models. This research aims to improve the understanding of the optical and microphysical properties of different types of aerosols particles. Samples of volcanic ash, Saharan dust and other mineral aerosols particles were analyzed by different techniques. Ground samples were sieved down to 45um, de-agglomerated and resuspended in the laboratory using a Fluidized Bed Aerosol Generator (FBAG). Particles were collected on Nuclepore filters into PM10, PM2.5, or PM1.0. and analyzed by different techniques, such as Scanning Electron Microscopy (SEM) for determination of size distribution and shape, spectral reflectance for determination of the optical absorption properties as a function of the wavelength, material density, and X-Ray fluorescence for the elemental composition. The spectral imaginary part of refractive index from the UV to the short wave infrared (SWIR) wavelength was derived empirically from the measurements of the spectral mass absorption coefficient, size distribution and density of the material. Some selected samples were also analyzed with the Polarized Imaging Nephelometer (PI-Neph) instrument for the characterization of the aerosol polarized phase function. This work compares results of the spectral refractive index of different materials obtained by our methodology with those available in the literature. In some cases there are significant differences both in magnitude and spectral dependence of the imaginary refractive index. These differences are evaluated and discussed in this work.

  9. Classifying aerosol type using in situ surface spectral aerosol optical properties

    NASA Astrophysics Data System (ADS)

    Schmeisser, Lauren; Andrews, Elisabeth; Ogren, John A.; Sheridan, Patrick; Jefferson, Anne; Sharma, Sangeeta; Kim, Jeong Eun; Sherman, James P.; Sorribas, Mar; Kalapov, Ivo; Arsov, Todor; Angelov, Christo; Mayol-Bracero, Olga L.; Labuschagne, Casper; Kim, Sang-Woo; Hoffer, András; Lin, Neng-Huei; Chia, Hao-Ping; Bergin, Michael; Sun, Junying; Liu, Peng; Wu, Hao

    2017-10-01

    Knowledge of aerosol size and composition is important for determining radiative forcing effects of aerosols, identifying aerosol sources and improving aerosol satellite retrieval algorithms. The ability to extrapolate aerosol size and composition, or type, from intensive aerosol optical properties can help expand the current knowledge of spatiotemporal variability in aerosol type globally, particularly where chemical composition measurements do not exist concurrently with optical property measurements. This study uses medians of the scattering Ångström exponent (SAE), absorption Ångström exponent (AAE) and single scattering albedo (SSA) from 24 stations within the NOAA/ESRL Federated Aerosol Monitoring Network to infer aerosol type using previously published aerosol classification schemes.Three methods are implemented to obtain a best estimate of dominant aerosol type at each station using aerosol optical properties. The first method plots station medians into an AAE vs. SAE plot space, so that a unique combination of intensive properties corresponds with an aerosol type. The second typing method expands on the first by introducing a multivariate cluster analysis, which aims to group stations with similar optical characteristics and thus similar dominant aerosol type. The third and final classification method pairs 3-day backward air mass trajectories with median aerosol optical properties to explore the relationship between trajectory origin (proxy for likely aerosol type) and aerosol intensive parameters, while allowing for multiple dominant aerosol types at each station.The three aerosol classification methods have some common, and thus robust, results. In general, estimating dominant aerosol type using optical properties is best suited for site locations with a stable and homogenous aerosol population, particularly continental polluted (carbonaceous aerosol), marine polluted (carbonaceous aerosol mixed with sea salt) and continental dust/biomass sites

  10. Chemical properties and outflow patterns of anthropogenic and dust particles on Rishiri Island during the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia)

    NASA Astrophysics Data System (ADS)

    Matsumoto, Kiyoshi; Uyama, Yukiko; Hayano, Teruaki; Tanimoto, Hiroshi; Uno, Itsushi; Uematsu, Mitsuo

    2003-12-01

    Investigations of chemical properties and transport mechanisms of continental aerosols are necessary for estimating their influences on global radiative budget and on the global material cycle. Intensive measurements of atmospheric aerosols and the associated species on Rishiri Island, near the northern tip of Japan, were conducted from March to May 2001, in order to understand the chemical properties, source regions, transport pathways, and transport patterns of anthropogenic and mineral aerosols over the east Asian Pacific Rim region during the spring. Mean concentrations of nss-SO42-, NO3-, NH4+, nss-Ca2+ in aerosols were 2.48, 0.64, 0.72, and 0.17 μg m-3, respectively. Elemental carbon and organic carbon in fine particles (d < 2.5 μm) yielded mean concentrations of 0.25 and 0.80 μg m-3, respectively. The concentrations of these species frequently increased to higher values because of outbreaks of continental polluted air masses, whereas under background conditions, they decreased to lower values similar to those observed over the remote ocean. Our results demonstrate that nss-SO42- and NH4+ coexist in fine particles, that NO3- and nss-Ca2+ coexist in coarse particles, and that each set is transported in an alternate manner. Continentally derived NO3- is transported as coarse particle to the east Asian Pacific Rim region. Anthropogenic pollutants and dust particles are not necessarily transported together. It was often found that anthropogenic fine particles containing abundant nss-SO42- appeared first and were then followed by large mineral particles that had absorbed NO3-. Short-term intrusion of the air masses containing abundant particulate carbonaceous compounds, probably due to the influence of biomass burning, also often occurred during the outflow events of continental air masses. Atmospheric behaviors of sulfate, nitrate, and carbonaceous species are different from one another, although they are all derived mainly from combustion processes.

  11. An Automated Method of MFRSR Calibration for Aerosol Optical Depth Analysis with Application to an Asian Dust Outbreak over the United States.

    NASA Astrophysics Data System (ADS)

    Augustine, John A.; Cornwall, Christopher R.; Hodges, Gary B.; Long, Charles N.; Medina, Carlos I.; Deluisi, John J.

    2003-02-01

    Over the past decade, networks of Multifilter Rotating Shadowband Radiometers (MFRSR) and automated sun photometers have been established in the United States to monitor aerosol properties. The MFRSR alternately measures diffuse and global irradiance in six narrow spectral bands and a broadband channel of the solar spectrum, from which the direct normal component for each may be inferred. Its 500-nm channel mimics sun photometer measurements and thus is a source of aerosol optical depth information. Automatic data reduction methods are needed because of the high volume of data produced by the MFRSR. In addition, these instruments are often not calibrated for absolute irradiance and must be periodically calibrated for optical depth analysis using the Langley method. This process involves extrapolation to the signal the MFRSR would measure at the top of the atmosphere (I0). Here, an automated clear-sky identification algorithm is used to screen MFRSR 500-nm measurements for suitable calibration data. The clear-sky MFRSR measurements are subsequently used to construct a set of calibration Langley plots from which a mean I0 is computed. This calibration I0 may be subsequently applied to any MFRSR 500-nm measurement within the calibration period to retrieve aerosol optical depth. This method is tested on a 2-month MFRSR dataset from the Table Mountain NOAA Surface Radiation Budget Network (SURFRAD) station near Boulder, Colorado. The resultant I0 is applied to two Asian dust-related high air pollution episodes that occurred within the calibration period on 13 and 17 April 2001. Computed aerosol optical depths for 17 April range from approximately 0.30 to 0.40, and those for 13 April vary from background levels to >0.30. Errors in these retrievals were estimated to range from ±0.01 to ±0.05, depending on the solar zenith angle. The calculations are compared with independent MFRSR-based aerosol optical depth retrievals at the Pawnee National Grasslands, 85 km to the

  12. Light absorbing material (soot) in rainwater and in aerosol particles in the Maldives

    NASA Astrophysics Data System (ADS)

    Granat, L.; EngströM, J. E.; Praveen, S.; Rodhe, H.

    2010-08-01

    Simultaneous measurements of soot (absorbing material at 528 nm) and inorganic ions in aerosol and precipitation at the Maldives Climate Observatory Hanimaadhoo during the period May 2005 to February 2007 have made it possible to calculate the washout ratio (WR) of these components as a measure of how efficiently they are scavenged by precipitation. On the basis of air trajectories the data have been separated into days with polluted air arriving from the Indian subcontinent in a northeasterly sector during winter and clean monsoon days with southerly flow from the Indian Ocean. The average soot concentration was a factor of 10 higher in the former situations. Despite considerable scatter for individual days, a systematic pattern emerged when the WR for the different components were compared with each other. During the monsoon season the WR for soot was similar to that of sulfate and other fine mode aerosol components, indicating that soot containing particles in these situations were efficient as cloud condensation nuclei. The origin of the light absorbing material during the monsoon season is unclear. During the polluted winter days, on the other hand, the WR for soot was three times smaller than that of sulfate. This indicates that, even after a travel time of several days, the soot containing particles from India have retained much of their hydrophobic property. The low WR and the infrequent rain during this season probably contribute to extending the atmospheric lifetime of soot well beyond several days. Surprisingly high concentrations of non-sea-salt calcium were measured during the monsoon season, substantially higher than during the winter season. The origin of these high values could be long-range transport from the Australian or African continents. Another possibility might be exopolymer gels derived from the ocean surface microlayer.

  13. Aerosol Optical Depth spatiotemporal variability and contribution of different aerosol types over Eastern Mediterranean

    NASA Astrophysics Data System (ADS)

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos; Zanis, Prodromos; Pöschl, Ulrich; Lelieveld, Jos; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios; Pozzer, Andrea

    2015-04-01

    In this work, we study the aerosol spatiotemporal variability over the region of Eastern Mediterranean, for the time period 2000-2012, using a 0.1-degree gridded dataset compiled from level-2 MODIS TERRA and MODIS AQUA AOD550 and FMR550 data. A detailed validation of the AOD550 data was implemented using ground-based observations from the AERONET, also showing that the gridding methodology we followed allows for the detection of several local hot spots that cannot be seen using lower resolutions or level-3 data. By combining the MODIS data with data from other satellite sensors (TOMS, OMI), data from a global chemical-aerosol-transport model (GOCART), and reanalysis data from MACC and ERA-interim, we quantify the relative contribution of different aerosol types to the total AOD550 for the period of interest. For this reason, we developed an optimized algorithm for regional studies based on results from previous global studies. Over land, anthropogenic, dust, and fine-mode natural aerosols contribute to the total AOD550, while anthropogenic, dust and maritime AODs are calculated over the ocean. The dust AOD550 over the region was compared against dust AODs from the LIVAS CALIPSO product, showing a similar seasonal variability. Finally, we also look into the aerosol load short-term trends over the region for each aerosol type separately, the results being strongly affected by the selected time period. The research leading to these results has received funding from the European Social Fund (ESF) and national resources under the operational programme Education and Lifelong Learning (EdLL) within the framework of the Action "Supporting Postdoctoral Researchers" (QUADIEEMS project) and from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement no. 226144 (C8 project).

  14. Potential of polarization lidar to provide profiles of CCN- and INP-relevant aerosol parameters

    NASA Astrophysics Data System (ADS)

    Mamouri, R. E.; Ansmann, A.

    2015-12-01

    We investigate the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nucleus (CCN) and ice nucleating particle (INP) number concentrations can be estimated. We show that height profiles of number concentrations of aerosol particles with radius > 50 nm (APC50, reservoir of favorable CCN) and with radius > 250 nm (APC250, reservoir of favorable INP), as well as profiles of the aerosol particle surface area concentration (ASC, used in INP parameterization) can be retrieved from lidar-derived aerosol extinction coefficients (AEC) with relative uncertainties of a factor of around 2 (APC50), and of about 25-50 % (APC250, ASC). Of key importance is the potential of polarization lidar to identify mineral dust particles and to distinguish and separate the aerosol properties of basic aerosol types such as mineral dust and continental pollution (haze, smoke). We investigate the relationship between AEC and APC50, APC250, and ASC for the main lidar wavelengths of 355, 532 and 1064 nm and main aerosol types (dust, pollution, marine). Our study is based on multiyear Aerosol Robotic Network (AERONET) photometer observations of aerosol optical thickness and column-integrated particle size distribution at Leipzig, Germany, and Limassol, Cyprus, which cover all realistic aerosol mixtures of continental pollution, mineral dust, and marine aerosol. We further include AERONET data from field campaigns in Morocco, Cabo Verde, and Barbados, which provide pure dust and pure marine aerosol scenarios. By means of a simple relationship between APC50 and the CCN-reservoir particles (APCCCN) and published INP parameterization schemes (with APC250 and ASC as input) we finally compute APCCCN and INP concentration profiles. We apply the full methodology to a lidar observation of a heavy dust outbreak crossing Cyprus with dust up to 8 km height and to a case during which anthropogenic pollution dominated.

  15. Asian Dust Storm Outbreaks: A Satellite-Surface Perspective

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee

    2006-01-01

    Airborne dusts from northern China contribute a significant part of the air quality problem and, to some extent, regional climatic impact in Asia during springtime. Asian dust typically originates in desert areas far from polluted urban regions. During the transport, dust layers can interact with anthropogenic sulfate and soot aerosols from heavily polluted urban areas. Added to the complex effects of clouds and natural marine aerosols, dust particles reaching the marine environment can have drastically different properties than those from the source. Thus, understanding the unique temporal and spatial variations of Asian dust is of special importance in regional-to-global climate issues (e.g., radiative forcing, hydrological cycle, and primary biological productivity in the mid-Pacific Ocean, etc.), as well as societal concerns (e.g., adverse health effects to humans). The Asian dust and air pollution aerosols can be detected by its colored appearance on current Earth observing satellites (e.g., MODIS, SeaWiFS, TOMS, etc.) and its evolution monitored by satellites and surface network (e.g. AERONET, SKY NET, MPLNET, etc.). Recently, many field campaigns (e.g., ACE-Asia-2001, TRACEP-2001, ADE-2002 & -2003, APEX-2001 & -2003, etc.) were designed and executed to study the compelling variability in spatial and temporal scale of both pollution-derived and naturally occurring aerosols, which often exist in high concentrations over eastern Asia and along the rim of the western Pacific. I will present an overview of the outbreak of Asian dust storms from space and surface observations and to address the climatic effects and societal impacts.

  16. The Fate of Saharan Dust Across the Atlantic and Implications for a Central American Dust Barrier

    NASA Technical Reports Server (NTRS)

    Nowottnick, E.; Colarco, P.; da Silva, A.; Hlavka, D.; McGill, M.

    2011-01-01

    Saharan dust was observed over the Caribbean basin during the summer 2007 NASA Tropical Composition, Cloud, and Climate Coupling (TC4) field experiment. Airborne Cloud Physics Lidar (CPL) and satellite observations from MODIS suggest a barrier to dust transport across Central America into the eastern Pacific. We use the NASA GEOS-5 atmospheric transport model with online aerosol tracers to perform simulations of the TC4 time period in order to understand the nature of this barrier. Our simulations are driven by the Modem Era Retrospective-Analysis for Research and Applications (MERRA) meteorological analyses. We evaluate our baseline simulated dust distributions using MODIS and CALIOP satellite and ground-based AERONET sun photometer observations. GEOS-5 reproduces the observed location, magnitude, and timing of major dust events, but our baseline simulation does not develop as strong a barrier to dust transport across Central America as observations suggest. Analysis of the dust transport dynamics and lost processes suggest that while both mechanisms play a role in defining the dust transport barrier, loss processes by wet removal of dust are about twice as important as transport. Sensitivity analyses with our model showed that the dust barrier would not exist without convective scavenging over the Caribbean. The best agreement between our model and the observations was obtained when dust wet removal was parameterized to be more aggressive, treating the dust as we do hydrophilic aerosols.

  17. Effect of Aerosols on Surface Radiation and Air Quality in the Central American Region Estimated Using Satellite UV Instruments

    NASA Astrophysics Data System (ADS)

    Bhartia, P. K.; Torres, O.; Krotkov, N. A.

    2007-05-01

    Solar radiation reaching the Earth's surface is reduced by both aerosol scattering and aerosol absorption. Over many parts of the world the latter effect can be as large or larger than the former effect, and small changes in the aerosol single scattering albedo can either cancel the former effect or enhance it. In addition, absorbing aerosols embedded in clouds can greatly reduce the amount of radiation reaching the surface by multiple scattering. Though the potential climatic effects of absorbing aerosols have received considerable attention lately, their effect on surface UV, photosynthesis, and photochemistry can be equally important for our environment and may affect human health and agricultural productivity. Absorption of all aerosols commonly found in the Earth's atmosphere becomes larger in the UV and blue wavelengths and has a relatively strong wavelength dependence. This is particularly true of mineral dust and organic aerosols. However, these effects have been very difficult to estimate on a global basis since the satellite instruments that operate in the visible are primarily sensitive to aerosol scattering. A notable exception is the UV Aerosol Index (AI), first produced using NASA's Nimbus-7 TOMS data. AI provides a direct measure of the effect of aerosol absorption on the backscattered UV radiation in both clear and cloudy conditions, as well as over snow/ice. Although many types of aerosols produce a distinct color cast in the visible images, and aerosols absorption over clouds and snow/ice could, in principle be detected from their color, so far this technique has worked well only in the UV. In this talk we will discuss what we have learned from the long-term record of AI produced from TOMS and Aura/OMI about the possible role of aerosols on surface radiation and air quality in the Central American region.

  18. Influences of natural emission sources (wildfires and Saharan dust) on the urban organic aerosol in Barcelona (Western Mediterranean Basis) during a PM event.

    PubMed

    van Drooge, Barend L; Lopez, Jordi F; Grimalt, Joan O

    2012-11-01

    The urban air quality in Barcelona in the Western Mediterranean Basin is characterized by overall high particulate matter (PM) concentrations, due to intensive local anthropogenic emissions and specific meteorological conditions. Moreover, on several days, especially in summer, natural PM sources, such as long-range transported Saharan dust from Northern Africa or wildfires on the Iberian Peninsula and around the Mediterranean Basin, may influence the levels and composition of the organic aerosol. In the second half of July 2009, daily collected PM(10) filter samples in an urban background site in Barcelona were analyzed on organic tracer compounds representing several emission sources. During this period, an important PM peak event was observed. Individual organic compound concentrations increased two to five times during this event. Although highest increase was observed for the organic tracer of biomass burning, the contribution to the organic aerosol was estimated to be around 6 %. Organic tracers that could be related to Saharan dust showed no correlation with the PM and OC levels, while this was the case for those related to fossil fuel combustion from traffic emissions. Moreover, a change in the meteorological conditions gave way to an overall increase of the urban background contamination. Long-range atmospheric transport of organic compounds from primary emissions sources (i.e., wildfires and Saharan dust) has a relatively moderate impact on the organic aerosol in an urban area where the local emissions are dominating.

  19. Dust Composition in Climate Models: Current Status and Prospects

    NASA Astrophysics Data System (ADS)

    Pérez García-Pando, C.; Miller, R. L.; Perlwitz, J. P.; Kok, J. F.; Scanza, R.; Mahowald, N. M.

    2015-12-01

    Mineral dust created by wind erosion of soil particles is the dominant aerosol by mass in the atmosphere. It exerts significant effects on radiative fluxes, clouds, ocean biogeochemistry, and human health. Models that predict the lifecycle of mineral dust aerosols generally assume a globally uniform mineral composition. However, this simplification limits our understanding of the role of dust in the Earth system, since the effects of dust strongly depend on the particles' physical and chemical properties, which vary with their mineral composition. Hence, not only a detailed understanding of the processes determining the dust emission flux is needed, but also information about its size dependent mineral composition. Determining the mineral composition of dust aerosols is complicated. The largest uncertainty derives from the current atlases of soil mineral composition. These atlases provide global estimates of soil mineral fractions, but they are based upon massive extrapolation of a limited number of soil samples assuming that mineral composition is related to soil type. This disregards the potentially large variability of soil properties within each defined soil type. In addition, the analysis of these soil samples is based on wet sieving, a technique that breaks the aggregates found in the undisturbed parent soil. During wind erosion, these aggregates are subject to partial fragmentation, which generates differences on the size distribution and composition between the undisturbed parent soil and the emitted dust aerosols. We review recent progress on the representation of the mineral and chemical composition of dust in climate models. We discuss extensions of brittle fragmentation theory to prescribe the emitted size-resolved dust composition, and we identify key processes and uncertainties based upon model simulations and an unprecedented compilation of observations.

  20. Aerosol Optical Depth Over India

    NASA Astrophysics Data System (ADS)

    David, Liji Mary; Ravishankara, A. R.; Kodros, John K.; Venkataraman, Chandra; Sadavarte, Pankaj; Pierce, Jeffrey R.; Chaliyakunnel, Sreelekha; Millet, Dylan B.

    2018-04-01

    Tropospheric aerosol optical depth (AOD) over India was simulated by Goddard Earth Observing System (GEOS)-Chem, a global 3-D chemical-transport model, using SMOG (Speciated Multi-pOllutant Generator from Indian Institute of Technology Bombay) and GEOS-Chem (GC) (current inventories used in the GEOS-Chem model) inventories for 2012. The simulated AODs were 80% (SMOG) and 60% (GC) of those measured by the satellites (Moderate Resolution Imaging Spectroradiometer and Multi-angle Imaging SpectroRadiometer). There is no strong seasonal variation in AOD over India. The peak AOD values are observed/simulated during summer. The simulated AOD using SMOG inventory has particulate black and organic carbon AOD higher by a factor 5 and 3, respectively, compared to GC inventory. The model underpredicted coarse-mode AOD but agreed for fine-mode AOD with Aerosol Robotic Network data. It captured dust only over Western India, which is a desert, and not elsewhere, probably due to inaccurate dust transport and/or noninclusion of other dust sources. The calculated AOD, after dust correction, showed the general features in its observed spatial variation. Highest AOD values were observed over the Indo-Gangetic Plain followed by Central and Southern India with lowest values in Northern India. Transport of aerosols from Indo-Gangetic Plain and Central India into Eastern India, where emissions are low, is significant. The major contributors to total AOD over India are inorganic aerosol (41-64%), organic carbon (14-26%), and dust (7-32%). AOD over most regions of India is a factor of 5 or higher than over the United States.

  1. Estimate of the Impact of Absorbing Aerosol Over Cloud on the MODIS Retrievals of Cloud Optical Thickness and Effective Radius Using Two Independent Retrievals of Liquid Water Path

    NASA Technical Reports Server (NTRS)

    Wilcox, Eric M.; Harshvardhan; Platnick, Steven

    2009-01-01

    Two independent satellite retrievals of cloud liquid water path (LWP) from the NASA Aqua satellite are used to diagnose the impact of absorbing biomass burning aerosol overlaying boundary-layer marine water clouds on the Moderate Resolution Imaging Spectrometer (MODIS) retrievals of cloud optical thickness (tau) and cloud droplet effective radius (r(sub e)). In the MODIS retrieval over oceans, cloud reflectance in the 0.86-micrometer and 2.13-micrometer bands is used to simultaneously retrieve tau and r(sub e). A low bias in the MODIS tau retrieval may result from reductions in the 0.86-micrometer reflectance, which is only very weakly absorbed by clouds, owing to absorption by aerosols in cases where biomass burning aerosols occur above water clouds. MODIS LWP, derived from the product of the retrieved tau and r(sub e), is compared with LWP ocean retrievals from the Advanced Microwave Scanning Radiometer-EOS (AMSR-E), determined from cloud microwave emission that is transparent to aerosols. For the coastal Atlantic southern African region investigated in this study, a systematic difference between AMSR-E and MODIS LWP retrievals is found for stratocumulus clouds over three biomass burning months in 2005 and 2006 that is consistent with above-cloud absorbing aerosols. Biomass burning aerosol is detected using the ultraviolet aerosol index from the Ozone Monitoring Instrument (OMI) on the Aura satellite. The LWP difference (AMSR-E minus MODIS) increases both with increasing tau and increasing OMI aerosol index. During the biomass burning season the mean LWP difference is 14 g per square meters, which is within the 15-20 g per square meter range of estimated uncertainties in instantaneous LWP retrievals. For samples with only low amounts of overlaying smoke (OMI AI less than or equal to 1) the difference is 9.4, suggesting that the impact of smoke aerosols on the mean MODIS LWP is 5.6 g per square meter. Only for scenes with OMI aerosol index greater than 2 does the

  2. [Aerosol optical properties during different air-pollution episodes over Beijing].

    PubMed

    Shi, Chan-Zhen; Yu, Xing-Na; Zhou, Bin; Xiang, Lei; Nie, Hao-Hao

    2013-11-01

    Based on the 2005-2011 data from Aerosol Robotic Network (AERONET), this study conducted analysis on aerosol optical properties over Beijing during different air-pollution episodes (biomass burning, CNY firework, dust storm). The aerosol optical depth (AOD) showed notable increases in the air-pollution episodes while the AOD (at 440 nm) during dust storm was 4. 91, 4. 07 and 2.65 times higher as background, biomass burning and firework aerosols. AOD along with Angstrom exponent (alpha) can be used to determine the aerosol types. The dust aerosol had the highest AOD and the lowest alpha. The alpha value of firework (1.09) was smaller than biomass burning (1.21) and background (1.27), indicating that coarse particles were dominant in the former type. Higher AOD of burnings (than background) can be attributed to the optical extinction capability of black carbon aerosol. The single scattering albedo (SSA) was insensitive to wavelength. The SSA value of dust (0.934) was higher than background (0.878), biomass burning (0.921) and firework (0.905). Additionally, the extremely large SSA of burnings here maybe was caused by the aging smoke, hygroscopic growth and so on. The peak radius of aerosol volume size distributions were 0.1-0.2 microm and 2.24 -3.85 microm in clear and polluted conditions. The value of volume concentration ratio between coarse and fine particles was in the order of clear background (1.04), biomass burning (1.10), CNY firework (1.91) and dust storm (4.96) episode.

  3. Mixing of Dust and NH3 Observed Globally over Anthropogenic Dust Sources

    NASA Technical Reports Server (NTRS)

    Ginoux, P.; Clarisse, L.; Clerbaux, C.; Coheur, P.-F.; Dubovik, O.; Hsu, N. C.; Van Damme, M.

    2012-01-01

    The global distribution of dust column burden derived from MODIS Deep Blue aerosol products is compared to NH3 column burden retrieved from IASI infrared spectra. We found similarities in their spatial distributions, in particular their hot spots are often collocated over croplands and to a lesser extent pastures. Globally, we found 22% of dust burden collocated with NH3, with only 1% difference between land-use databases. This confirms the importance of anthropogenic dust from agriculture. Regionally, the Indian subcontinent has the highest amount of dust mixed with NH3 (26 %), mostly over cropland and during the pre-monsoon season. North Africa represents 50% of total dust burden but accounts for only 4% of mixed dust, which is found over croplands and pastures in Sahel and the coastal region of the Mediterranean. In order to evaluate the radiative effect of this mixing on dust optical properties, we derive the mass extinction efficiency for various mixtures of dust and NH3, using AERONET sunphotometers data. We found that for dusty days the coarse mode mass extinction efficiency decreases from 0.62 to 0.48 square meters per gram as NH3 burden increases from 0 to 40 milligrams per square meter. The fine mode extinction efficiency, ranging from 4 to 16 square mters per gram, does not appear to depend on NH3 concentration or relative humidity but rather on mineralogical composition and mixing with other aerosols. Our results imply that a significant amount of dust is already mixed with ammonium salt before its long range transport. This in turn will affect dust lifetime, and its interactions with radiation and cloud properties

  4. Aerosol-Cloud-Precipitation Interactions over Indo-Gangetic Basin

    NASA Technical Reports Server (NTRS)

    Tsay, S.-C.; Lau, K. .; Holben, B. N.; Hsu, N. C.; Bhartia, P. K.

    2005-01-01

    About 60% of world population reside in Asia, in term of which sheer population density presents a major environmental stress. Economic expansion in this region is, in fact, accompanied by increases in bio-fuel burning, industrial pollution, and land cover and land use changes. With a growth rate of approx. 8%/yr for Indian economy, more than 600 million people from Lahore, Pakistan to Calcutta, India over the Indo-Gangetic Basin have particularly witnessed increased frequencies of floods and droughts as well as a dramatic increase in atmospheric loading of aerosols (i.e., anthropogenic and natural aerosol) in recent decades. This regional change (e.g., aerosol, cloud, precipitation, etc.) will constitute a vital part of the global change in the 21st century. Better understanding of the impacts of aerosols in affecting monsoon climate and water cycles is crucial in providing the physical basis to improve monsoon climate prediction and for disaster mitigation. Based on climate model simulations, absorbing aerosols (dust and black carbon) play a critical role in affecting interannual and intraseasonal variability of the Indian monsoon. An initiative on the integrated (aerosols, clouds, and precipitation) measurements approach over the Indo-Gangetic Basin will be discussed. An array of ground-based (e.g., AERONET, MPLNET, SMART-COMMIT, etc.) and satellite (e.g., Terra, A-Train, etc.) sensors will be utilized to acquire aerosol characteristics, sources/sinks, and transport processes during the pre-monsoon (April-May, aerosol forcing) season, and to obtain cloud and precipitation properties during the monsoon (May-June, water cycle response) season. Close collaboration with other international programs, such as ABC, CLIVAR, GEWEX, and CEOP in the region is anticipated.

  5. Using NASA EOS in the Arabian and Saharan Deserts to Examine Dust Particle Size and Spectral Signature of Aerosols

    NASA Astrophysics Data System (ADS)

    Brenton, J. C.; Keeton, T.; Barrick, B.; Cowart, K.; Cooksey, K.; Florence, V.; Herdy, C.; Luvall, J. C.; Vasquez, S.

    2012-12-01

    Exposure to high concentrations of airborne particulate matter can have adverse effects on the human respiratory system. Ground-based studies conducted in Iraq have revealed the presence of potential human pathogens in airborne dust. According to the Environmental Protection Agency (EPA), airborne particulate matter below 2.5μm (PM2.5) can cause long-term damage to the human respiratory system. Given the relatively high incidence of new-onset respiratory disorders experienced by US service members deployed to Iraq, this research offers a new glimpse into how satellite remote sensing can be applied to questions related to human health. NASA's Earth Observing System (EOS) can be used to determine spectral characteristics of dust particles, the depth of dust plumes, as well as dust particle sizes. Comparing dust particle size from the Sahara and Arabian Deserts gives insight into the composition and atmospheric transport characteristics of dust from each desert. With the use of NASA SeaWiFS DeepBlue Aerosol, dust particle sizes were estimated using Angström exponent. Brightness Temperature Difference (BTD) equation was used to determine the distribution of particle sizes, the area of the dust storm, and whether silicate minerals were present in the dust. The Moderate-resolution Imaging Spectroradiometer (MODIS) on Terra satellite was utilized in calculating BTD. Minimal research has been conducted on the spectral characteristics of airborne dust in the Arabian and Sahara Deserts. Mineral composition of a dust storm that occurred 17 April 2008 near Baghdad was determined using imaging spectrometer data from the Jet Propulsion Laboratory Spectral Library and EO-1 Hyperion data. Mineralogy of this dust storm was subsequently compared to that of a dust storm that occurred over the Bodélé Depression in the Sahara Desert on 7 June 2003.

  6. Impacts of snow darkening by absorbing aerosols on South Asian monsoon

    NASA Astrophysics Data System (ADS)

    Kim, K. M.; Lau, W. K. M.; Kim, M. K.; Sang, J.; Yasunari, T. J.; Koster, R. D.

    2016-12-01

    Seasonal heating over the Tibetan Plateau is a main driver of the onset of the South Asian Monsoon. Aerosols can play an important role in pre- and early monsoon seasonal heating process over the Tibetan Plateau by increasing atmospheric heating in the northern India, and by heating of the surface of the Tibetan Plateau and Himalayan slopes, via reduction of albedo of the snow surface through surface deposition - the so call snow-darkening effect (SDE). To examine the impact of SDE on weather and climate during late spring and early summer, two sets of NASA/GEOS-5 model simulations with and without SDE are conducted. Results show that SDE-induced surface heating accelerates snow melts and increases surface temperature over 4K in the entire Tibetan Plateau regions during boreal summer. Warmer Tibetan Plateau further accelerates seasonal warming in the upper troposphere and increases the north-south temperature gradient between the Tibetan Plateau and the equatorial Indian Ocean. This reversal of the north-south temperature gradient is a primary cause of the onset of the South Asian monsoon. SDE-induced increase of the meridional temperature gradient drives meridional circulation and enhanced upper tropospheric easterlies and lower tropospheric westerlies, and intensifies monsoon circulation and rainfall. This pattern enhances the EHP-like circulation anomalies induced by atmospheric heating of absorbing aerosols over the northern India. SDE-induced change in the India subcontinent differs that in Eurasia. SDE-induced land-atmospheric interactions in two regions will be also compared.

  7. Determination of Monthly Aerosol Types in Manila Observatory and Notre Dame of Marbel University from Aerosol Robotic Network (AERONET) measurements.

    NASA Astrophysics Data System (ADS)

    Ong, H. J. J.; Lagrosas, N.; Uy, S. N.; Gacal, G. F. B.; Dorado, S.; Tobias, V., Jr.; Holben, B. N.

    2016-12-01

    This study aims to identify aerosol types in Manila Observatory (MO) and Notre Dame of Marbel University (NDMU) using Aerosol Robotic Network (AERONET) Level 2.0 inversion data and five dimensional specified clustering and Mahalanobis classification. The parameters used are the 440-870 nm extinction Angström exponent (EAE), 440 nm single scattering albedo (SSA), 440-870 nm absorption Angström exponent (AAE), 440 nm real and imaginary refractive indices. Specified clustering makes use of AERONET data from 7 sites to define 7 aerosol classes: mineral dust (MD), polluted dust (PD), urban industrial (UI), urban industrial developing (UID), biomass burning white smoke (BBW), biomass burning dark smoke (BBD), and marine aerosols. This is similar to the classes used by Russell et al, 2014. A data point is classified into a class based on the closest 5-dimensional Mahalanobis distance (Russell et al, 2014 & Hamill et al, 2016). This method is applied to all 173 MO data points from January 2009 to June 2015 and to all 24 NDMU data points from December 2009 to July 2015 to look at monthly and seasonal variations of aerosol types. The MO and NDMU aerosols are predominantly PD ( 77%) and PD & UID ( 75%) respectively (Figs.1a-b); PD is predominant in the months of February to May in MO and February to March in NDMU. PD results from less strict emission and environmental regulations (Catrall 2005). Average SSA values in MO is comparable to the mean SSA for PD ( 0.89). This can be attributed to presence of high absorbing aerosol types, e.g., carbon which is a product of transportation emissions. The second most dominant aerosol type in MO is UID ( 15%), in NDMU it is BBW ( 25%). In Manila, the high sources of PD and UID (fine particles) is generally from vehicular combustion (Oanh, et al 2006). The detection of BBW in MO from April to May can be attributed to the fires which are common in these dry months. In NDMU, BBW source is from biomass burning (smoldering). In this

  8. Direct and semi-direct aerosol radiative effect on the Mediterranean climate variability using a coupled regional climate system model

    NASA Astrophysics Data System (ADS)

    Nabat, Pierre; Somot, Samuel; Mallet, Marc; Sevault, Florence; Chiacchio, Marc; Wild, Martin

    2015-02-01

    A fully coupled regional climate system model (CNRM-RCSM4) has been used over the Mediterranean region to investigate the direct and semi-direct effects of aerosols, but also their role in the radiation-atmosphere-ocean interactions through multi-annual ensemble simulations (2003-2009) with and without aerosols and ocean-atmosphere coupling. Aerosols have been taken into account in CNRM-RCSM4 through realistic interannual monthly AOD climatologies. An evaluation of the model has been achieved, against various observations for meteorological parameters, and has shown the ability of CNRM-RCSM4 to reproduce the main patterns of the Mediterranean climate despite some biases in sea surface temperature (SST), radiation and cloud cover. The results concerning the aerosol radiative effects show a negative surface forcing on average because of the absorption and scattering of the incident radiation. The SW surface direct effect is on average -20.9 Wm-2 over the Mediterranean Sea, -14.7 Wm-2 over Europe and -19.7 Wm-2 over northern Africa. The LW surface direct effect is weaker as only dust aerosols contribute (+4.8 Wm-2 over northern Africa). This direct effect is partly counterbalanced by a positive semi-direct radiative effect over the Mediterranean Sea (+5.7 Wm-2 on average) and Europe (+5.0 Wm-2) due to changes in cloud cover and atmospheric circulation. The total aerosol effect is consequently negative at the surface and responsible for a decrease in land (on average -0.4 °C over Europe, and -0.5 °C over northern Africa) and sea surface temperature (on average -0.5 °C for the Mediterranean SST). In addition, the latent heat loss is shown to be weaker (-11.0 Wm-2) in the presence of aerosols, resulting in a decrease in specific humidity in the lower troposphere, and a reduction in cloud cover and precipitation. Simulations also indicate that dust aerosols warm the troposphere by absorbing solar radiation, and prevent radiation from reaching the surface, thus

  9. Utilization of O4 Slant Column Density to Derive Aerosol Layer Height from a Spaceborne UV-Visible Hyperspectral Sensor: Sensitivity and Case Study

    NASA Technical Reports Server (NTRS)

    Park, Sang Seo; Kim, Jhoon; Lee, Hanlim; Torres, Omar; Lee, Kwang-Mog; Lee, Sang Deok

    2016-01-01

    The sensitivities of oxygen-dimer (O4) slant column densities (SCDs) to changes in aerosol layer height are investigated using the simulated radiances by a radiative transfer model, the linearized pseudo-spherical vector discrete ordinate radiative transfer (VLIDORT), and the Differential Optical Absorption Spectroscopy (DOAS) technique. The sensitivities of the O4 index (O4I), which is defined as dividing O4 SCD by 10(exp 40) sq molecules cm(exp -5), to aerosol types and optical properties are also evaluated and compared. Among the O4 absorption bands at 340, 360, 380, and 477 nm, the O4 absorption band at 477 nm is found to be the most suitable to retrieve the aerosol effective height. However, the O4I at 477 nm is significantly influenced not only by the aerosol layer effective height but also by aerosol vertical profiles, optical properties including single scattering albedo (SSA), aerosol optical depth (AOD), particle size, and surface albedo. Overall, the error of the retrieved aerosol effective height is estimated to be 1276, 846, and 739 m for dust, non-absorbing, and absorbing aerosol, respectively, assuming knowledge on the aerosol vertical distribution shape. Using radiance data from the Ozone Monitoring Instrument (OMI), a new algorithm is developed to derive the aerosol effective height over East Asia after the determination of the aerosol type and AOD from the MODerate resolution Imaging Spectroradiometer (MODIS). About 80% of retrieved aerosol effective heights are within the error range of 1 km compared to those obtained from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) measurements on thick aerosol layer cases.

  10. Predicting the mineral composition of dust aerosols: Insights from elemental composition measured at the Izaña Observatory

    NASA Astrophysics Data System (ADS)

    Pérez García-Pando, Carlos; Miller, Ron L.; Perlwitz, Jan P.; Rodríguez, Sergio; Prospero, Joseph M.

    2016-10-01

    Regional variations of dust mineral composition are fundamental to climate impacts but generally neglected in climate models. A challenge for models is that atlases of soil composition are derived from measurements following wet sieving, which destroys the aggregates potentially emitted from the soil. Aggregates are crucial to simulating the observed size distribution of emitted soil particles. We use an extension of brittle fragmentation theory in a global dust model to account for these aggregates. Our method reproduces the size-resolved dust concentration along with the approximately size-invariant fractional abundance of elements like Fe and Al in the decade-long aerosol record from the Izaña Observatory, off the coast of West Africa. By distinguishing between Fe in structural and free forms, we can attribute improved model behavior to aggregation of Fe and Al-rich clay particles. We also demonstrate the importance of size-resolved measurements along with elemental composition analysis to constrain models.

  11. Photochemical oxidant processes in the presence of dust: An evaluation of the impact of dust on particulate nitrate and ozone formation

    NASA Technical Reports Server (NTRS)

    Zhang, Yang; Sunwoo, Young; Kotamarthi, Veerabhadra; Carmichael, Gregory R.

    1994-01-01

    The influence of dust on the tropospheric photochemical oxidant cycle is studied through the use of a detailed coupled aerosol and gas-phase chemistry model. Dust is a significant component of the troposphere throughout Asia and provides a surface for a variety of heterogeneous reactions. Dust is found to be an important surface for particulate nitrate formation. For dust loading and ambient concentrations representative of conditions in East Asia, particulate nitrate levels of 1.5-11.5 micrograms/cubic meter are predicted, consistent with measured levels in this region. Dust is also found to reduce NO(x) levels by up to 50%, HO2 concentrations by 20%-80%, and ozone production rates by up to 25%. The magnitude of the influence of dust is sensitive to mass concentration of the aerosol, relative humidity, and the value of the accommodation coefficient.

  12. The early summertime Saharan heat low: sensitivity of the radiation budget and atmospheric heating to water vapour and dust aerosol

    NASA Astrophysics Data System (ADS)

    Alamirew, Netsanet K.; Todd, Martin C.; Ryder, Claire L.; Marsham, John H.; Wang, Yi

    2018-01-01

    The Saharan heat low (SHL) is a key component of the west African climate system and an important driver of the west African monsoon across a range of timescales of variability. The physical mechanisms driving the variability in the SHL remain uncertain, although water vapour has been implicated as of primary importance. Here, we quantify the independent effects of variability in dust and water vapour on the radiation budget and atmospheric heating of the region using a radiative transfer model configured with observational input data from the Fennec field campaign at the location of Bordj Badji Mokhtar (BBM) in southern Algeria (21.4° N, 0.9° E), close to the SHL core for June 2011. Overall, we find dust aerosol and water vapour to be of similar importance in driving variability in the top-of-atmosphere (TOA) radiation budget and therefore the column-integrated heating over the SHL (˜ 7 W m-2 per standard deviation of dust aerosol optical depth - AOD). As such, we infer that SHL intensity is likely to be similarly enhanced by the effects of dust and water vapour surge events. However, the details of the processes differ. Dust generates substantial radiative cooling at the surface (˜ 11 W m-2 per standard deviation of dust AOD), presumably leading to reduced sensible heat flux in the boundary layer, which is more than compensated by direct radiative heating from shortwave (SW) absorption by dust in the dusty boundary layer. In contrast, water vapour invokes a radiative warming at the surface of ˜ 6 W m-2 per standard deviation of column-integrated water vapour in kg m-2. Net effects involve a pronounced net atmospheric radiative convergence with heating rates on average of 0.5 K day-1 and up to 6 K day-1 during synoptic/mesoscale dust events from monsoon surges and convective cold-pool outflows (haboobs). On this basis, we make inferences on the processes driving variability in the SHL associated with radiative and advective heating/cooling. Depending

  13. Interpreting the Ultraviolet Aerosol Index Observed with the OMI Satellite Instrument to Understand Absorption by Organic Aerosols: Implications for Atmospheric Oxidation and Direct Radiative Effects

    NASA Technical Reports Server (NTRS)

    Hammer, Melanie S.; Martin, Randall V.; Donkelaar, Aaron van; Buchard, Virginie; Torres, Omar; Ridley, David A.; Spurr, Robert J. D.

    2016-01-01

    Satellite observations of the ultraviolet aerosol index (UVAI) are sensitive to absorption of solar radiation by aerosols; this absorption affects photolysis frequencies and radiative forcing. We develop a global simulation of the UVAI using the 3-D chemical transport model GEOSChem coupled with the Vector Linearized Discrete Ordinate Radiative Transfer model (VLIDORT). The simulation is applied to interpret UVAI observations from the Ozone Monitoring Instrument (OMI) for the year 2007. Simulated and observed values are highly consistent in regions where mineral dust dominates the UVAI, but a large negative bias (-0.32 to -0.97) exists between simulated and observed values in biomass burning regions. We determine effective optical properties for absorbing organic aerosol, known as brown carbon (BrC), and implement them into GEOS-Chem to better represent observed UVAI values over biomass burning regions. The inclusion of absorbing BrC decreases the mean bias between simulated and OMI UVAI values from -0.57 to -0.09 over West Africa in January, from -0.32 to +0.0002 over South Asia in April, from -0.97 to -0.22 over southern Africa in July, and from -0.50 to +0.33 over South America in September. The spectral dependence of absorption after including BrC in the model is broadly consistent with reported observations for biomass burning aerosol, with absorbing Angstrom exponent (AAE) values ranging from 2.9 in the ultraviolet (UV) to 1.3 across the UV-Near IR spectrum. We assess the effect of the additional UV absorption by BrC on atmospheric photochemistry by examining tropospheric hydroxyl radical (OH) concentrations in GEOS-Chem. The inclusion of BrC decreases OH by up to 30% over South America in September, up to 20% over southern Africa in July, and up to 15% over other biomass burning regions. Global annual mean OH concentrations in GEOS-Chem decrease due to the presence of absorbing BrC, increasing the methyl chloroform lifetime from 5.62 to 5.68 years, thus

  14. Current Status of Aerosol Retrievals from TOMS

    NASA Technical Reports Server (NTRS)

    Torres, O.; Herman, J. R.; Bhartia, P. K.; Ginoux, P.

    1999-01-01

    Properties of atmospheric aerosols over all land and water surfaces are retrieved from TOMS measurements of backscattered radiances. The TOMS technique, uses observations at two wavelengths. In the near ultraviolet (330-380 nm) range, where the effects of gaseous absorption are negligible. The retrieved properties are optical depth and a measure of aerosol absorptivity, generally expressed as single scattering albedo. The main sources of error of the TOMS aerosol products are sub-pixel cloud contamination and uncertainty on the height above the surface of UV-absorbing aerosol layers. The first error source is related to the large footprint (50 x 50 km at nadir) of the sensor, and the lack of detection capability of sub-pixel size clouds. The uncertainty associated with the height of the absorbing aerosol layers, on the other hand, is related to the pressure dependence of the molecular scattering process, which is the basis of the near-UV method of absorbing aerosol detection. The detection of non-absorbing aerosols is not sensitive to aerosol layer height. We will report on the ongoing work to overcome both of these difficulties. Coincident measurements of high spatial resolution thermal infrared radiances are used to address the cloud contamination issue. Mostly clear scenes for aerosol retrieval are selected by examining the spatial homogeneity of the IR radiance measurements within a TOMS pixel. The approach to reduce the uncertainty associated with the height of the aerosol layer by making use of a chemical transport model will also be discussed.

  15. Assessment of the aerosol distribution over Indian subcontinent in CMIP5 models

    NASA Astrophysics Data System (ADS)

    Sanap, S. D.; Ayantika, D. C.; Pandithurai, G.; Niranjan, K.

    2014-04-01

    This paper examines the aerosol distribution over Indian subcontinent as represented in 21 models from Coupled Model Inter-comparison Project Phase 5 (CMIP5) simulations, wherein model simulated aerosol optical depth (AOD) is compared with Moderate Resolution Imaging Spectro-radiometer (MODIS) satellite observations. The objective of the study is to provide an assessment of the capability of various global models, participating in CMIP5 project, in capturing the realistic spatial and temporal distribution of aerosol species over the Indian subcontinent. Results from our analysis show that majority of the CMIP5 models (excepting HADGEM2-ES, HADGEM2-CC) seriously underestimates the spatio-temporal variability of aerosol species over the Indian subcontinent, in particular over Indo-Gangetic Plains (IGP). Since IGP region is dominated by anthropogenic activities, high population density, and wind driven transport of dust and other aerosol species, MODIS observations reveal high AOD values over this region. Though the representation of black carbon (BC) loading in many models is fairly good, the dust loading is observed to be significantly low in majority of the models. The presence of pronounced dust activity over northern India and dust being one of the major constituent of aerosol species, the biases in dust loading has a great impact on the AOD of that region. We found that considerable biases in simulating the 850 hPa wind field (which plays important role in transport of dust from adjacent deserts) would be the possible reason for poor representation of dust AOD and in turn total AOD over Indian region in CMIP5 models. In addition, aerosol radiative forcing (ARF) underestimated/overestimated in most of the models. However, spatial distribution of ARF in multi-model ensemble mean is comparable reasonably well with observations with bias in magnitudes. This analysis emphasizes the fundamental need to improve the representation of aerosol species in current state of

  16. Indirect estimation of absorption properties for fine aerosol particles using AATSR observations: a case study of wildfires in Russia in 2010

    NASA Astrophysics Data System (ADS)

    Rodriguez, E.; Kolmonen, P.; Virtanen, T. H.; Sogacheva, L.; Sundstrom, A.-M.; de Leeuw, G.

    2015-08-01

    The Advanced Along-Track Scanning Radiometer (AATSR) on board the ENVISAT satellite is used to study aerosol properties. The retrieval of aerosol properties from satellite data is based on the optimized fit of simulated and measured reflectances at the top of the atmosphere (TOA). The simulations are made using a radiative transfer model with a variety of representative aerosol properties. The retrieval process utilizes a combination of four aerosol components, each of which is defined by their (lognormal) size distribution and a complex refractive index: a weakly and a strongly absorbing fine-mode component, coarse mode sea salt aerosol and coarse mode desert dust aerosol). These components are externally mixed to provide the aerosol model which in turn is used to calculate the aerosol optical depth (AOD). In the AATSR aerosol retrieval algorithm, the mixing of these components is decided by minimizing the error function given by the sum of the differences between measured and calculated path radiances at 3-4 wavelengths, where the path radiances are varied by varying the aerosol component mixing ratios. The continuous variation of the fine-mode components allows for the continuous variation of the fine-mode aerosol absorption. Assuming that the correct aerosol model (i.e. the correct mixing fractions of the four components) is selected during the retrieval process, also other aerosol properties could be computed such as the single scattering albedo (SSA). Implications of this assumption regarding the ratio of the weakly/strongly absorbing fine-mode fraction are investigated in this paper by evaluating the validity of the SSA thus obtained. The SSA is indirectly estimated for aerosol plumes with moderate-to-high AOD resulting from wildfires in Russia in the summer of 2010. Together with the AOD, the SSA provides the aerosol absorbing optical depth (AAOD). The results are compared with AERONET data, i.e. AOD level 2.0 and SSA and AAOD inversion products. The RMSE

  17. The Saharan Aerosol Long-range Transport and Aerosol-Cloud-Interaction Experiment SALTRACE 2013 - Overview and Early Results (Invited)

    NASA Astrophysics Data System (ADS)

    Weinzierl, B.; Ansmann, A.; Reitebuch, O.; Freudenthaler, V.; Müller, T.; Kandler, K.; Althausen, D.; Busen, R.; Dollner, M.; Dörnbrack, A.; Farrell, D. A.; Gross, S.; Heimerl, K.; Klepel, A.; Kristensen, T. B.; Mayol-Bracero, O. L.; Minikin, A.; Prescod, D.; Prospero, J. M.; Rahm, S.; Rapp, M.; Sauer, D. N.; Schaefler, A.; Toledano, C.; Vaughan, M.; Wiegner, M.

    2013-12-01

    Mineral dust is an important player in the global climate system. In spite of substantial progress in the past decade, many questions in our understanding of the atmospheric and climate effects of mineral dust remain open such as the change of the dust size distribution during transport across the Atlantic Ocean and the associated impact on the radiation budget, the role of wet and dry dust removal mechanisms during transport, and the complex interaction between mineral dust and clouds. To close gaps in our understanding of mineral dust in the climate system, the Saharan Aerosol Long-range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE: http://www.pa.op.dlr.de/saltrace) was conducted in June/July 2013. SALTRACE is a German initiative combining ground-based and airborne in-situ and lidar measurements with meteorological data, long-term measurements, satellite remote sensing and modeling. During SALTRACE, the DLR research aircraft Falcon was based on Sal, Cape Verde, between 11 and 17 June, and on Barbados between 18 June and 11 July 2013. The Falcon was equipped with a suite of in-situ instruments for the measurement of microphysical and optical aerosol properties and with a nadir-looking 2-μm wind lidar. Ground-based lidar and in-situ instruments were deployed in Barbados and Puerto Rico. Mineral dust from several dust outbreaks was measured by the Falcon between Senegal and Florida. On the eastern side of the Atlantic, dust plumes extended up to 6 km altitude, while the dust layers in the Caribbean were mainly below 4.5 km. The aerosol optical thickness of the dust outbreaks studied ranged from 0.2 to 0.6 at 500 nm in Barbados. Highlights during SALTRACE included the sampling of a dust plume in the Cape Verde area on 17 June which was again measured with the same instrumentation on 21 and 22 June near Barbados. The event was also captured by the ground-based lidar and in-situ instrumentation. Another highlight was the formation of tropical storm

  18. Direct radiative effects induced by intense desert dust outbreaks over the broader Mediterranean basin

    NASA Astrophysics Data System (ADS)

    Gkikas, Antonis; Obiso, Vincenzo; Vendrell, Lluis; Basart, Sara; Jorba, Oriol; Pérez Garcia-Pando, Carlos; Hatzianastassiou, Nikos; Gassó, Santiago; Baldasano, Jose Maria

    2016-04-01

    Throughout the year, under favorable conditions, massive loads of mineral particles originating in the northern African and Middle East deserts are transported over the Mediterranean basin. Due to their composition and size, dust aerosols perturb the Earth-Atmosphere system's energy budget interacting directly with the shortwave (SW) and longwave (LW) radiation. The present study aims to compute the Mediterranean dust outbreaks' direct radiative effects (DREs) as well as to assess the effect of including dust DREs in numerical simulations of a regional model. To this aim, 20 intense dust outbreaks have been selected based on their spatial coverage and intensity. Their identification, over the period 2000-2013, has been achieved through an objective and dynamic algorithm which utilizes as inputs daily satellite retrievals derived by the MODIS-Terra, EP-TOMS and OMI-Aura sensors. For each outbreak, two simulations of the NMMB/BSC-Dust model were made for a forecast period of 84 hours, with the model initialized at 00 UTC of the day when the dust outbreak was ignited, activating (RADON) and deactivating (RADOFF) dust-radiation interactions. The simulation domain covers the northern Africa, the Middle East and Europe at 0.25° x 0.25° horizontal resolution, for 40 hybrid sigma pressure levels up to 50 hPa. The instantaneous and regional DREs have been calculated at the top of the atmosphere (TOA), into the atmosphere (ATMAB), and at surface, for the downwelling (SURF) and the absorbed (NETSURF) radiation, for the SW, LW and NET (SW+LW) radiation. The interaction between dust aerosols and NET radiation, locally leads to an atmospheric warming (DREATMAB) by up to 150 Wm-2, a surface cooling (DRENETSURF) by up to 250 Wm-2 and a reduction of the downwelling radiation at the surface (DRESURF) by up to 300 Wm-2. At TOA, DREs are mainly negative (down to -150 Wm-2) indicating a cooling of the Earth-Atmosphere system, although positive values (up to 50 Wm-2) are encountered

  19. Stratospheric aerosols and climatic change

    NASA Technical Reports Server (NTRS)

    Toon, O. B.; Pollack, J. B.

    1978-01-01

    Stratospht1ic sulfuric acid particles scatter and absorb sunlight and they scatter, absorb and emit terrestrial thermal radiation. These interactions play a role in the earth's radiation balance and therefore affect climate. The stratospheric aerosols are perturbed by volcanic injection of SO2 and ash, by aircraft injection of SO2, by rocket exhaust of Al2O3 and by tropospheric mixing of particles and pollutant SO2 and COS. In order to assess the effects of these perturbations on climate, the effects of the aerosols on the radiation balance must be understood and in order to understand the radiation effects the properties of the aerosols must be known. The discussion covers the aerosols' effect on the radiation balance. It is shown that the aerosol size distribution controls whether the aerosols will tend to warm or cool the earth's surface. Calculations of aerosol properties, including size distribution, for various perturbation sources are carried out on the basis of an aerosol model. Calculations are also presented of the climatic impact of perturbed aerosols due to volcanic eruptions and Space Shuttle flights.

  20. In Situ Observations of Snow Metamorphosis Acceleration Induced by Dust and Black Carbon

    NASA Astrophysics Data System (ADS)

    Schneider, A. M.; Flanner, M.

    2017-12-01

    Previous studies demonstrate the dependence of shortwave infrared (SWIR) reflectance on snow specific surface area (SSA) and others examine the direct darkening effect dust and black carbon (BC) deposition has on snow and ice-covered surfaces. The extent to which these light absorbing aerosols (LAAs) accelerate snow metamorphosis, however, is challenging to assess in situ as measurement techniques easily disturb snowpack. Here, we use two Near-Infrared Emitting Reflectance Domes (NERDs) to measure 1300 and 1550nm bidirectional reflectance factors (BRFs) of natural snow and experimental plots with added dust and BC. We obtain NERD measurements and subsequently collect and transport snow samples to the nearby U.S. Army Corps of Engineers' Cold Regions Research and Engineering Lab for micro computed tomography (micro-CT) analysis. Snow 1300 (1550) nm BRFs evolve from 0.6 (0.15) in fresh snow to 0.2 (0.03) after metamorphosis. Hourly-scale time evolving snow surface BRFs and SSA estimates from micro-CT reveal more rapid SWIR darkening and snow metamorphosis in contaminated versus natural plots. Cloudiness and high wind speeds can completely obscure these results if LAAs mobilize before absorbing enough radiant energy. These findings verify experimentally that dust and BC deposition can accelerate snow metamorphosis and enhance snow albedo feedback in sunny, calm weather conditions. Although quantifying the enhancement of snow albedo feedback induced by LAAs requires further surface temperature, solar irradiance, and impurity concentration measurements, this study provides experimental verification of positive feedback occurring where dust and BC accelerate snow metamorphosis.