Sample records for aerosol climatology project

  1. The MAC aerosol climatology

    NASA Astrophysics Data System (ADS)

    Kinne, S.

    2015-12-01

    Aerosol is highly diverse in space and time. And many different aerosol optical properties are needed (consistent to each other) for the determination of radiative effects. To sidestep a complex (and uncertain) aerosol treatment (emission to mass to optics) a monthly gridded climatology for aerosol properties has been developed. This MPI Aerosol Climatology (MAC) is strongly tied to observational statistics for aerosol column optical properties by AERONET (over land) and by MAN (over oceans). To fill spatial gaps, to address decadal change and to address vertical variability, these sparsely distributed local data are extended with central data of an ensemble of output from global models with complex aerosol modules. This data merging in performed for aerosol column amount (AOD), for aerosol size (AOD,fine) and for aerosol absorption (AAOD). The resulting MAC aerosol climatology is an example for the combination of high quality local observations with spatial, temporal and vertical context from model simulations.

  2. Toward Creating A Global Retrospective Climatology of Aerosol Properties

    NASA Technical Reports Server (NTRS)

    Curran, Robert J.; Mishchenko, Michael I.; Hansen, James E. (Technical Monitor)

    2000-01-01

    Tropospheric aerosols are thought to cause a significant direct and indirect climate forcing, but the magnitude of this forcing remains highly uncertain because of poor knowledge of global aerosol characteristics and their temporal changes. The standard long-term global product, the one-channel Advanced Very-High-Resolution Radiometer (AVHRR) aerosol optical thickness over the ocean, relies on a single predefined aerosol model and can be inaccurate in many cases. Furthermore, it provides no information on aerosol column number density, thus making it impossible to estimate the indirect aerosol effect on climate. Total Ozone Mapping Spectrometer (TOMS) data can be used to detect absorbing aerosols over land, but are insensitive to aerosols located below one kilometer. It is thus clear that innovative approaches must be employed in order to extract a more quantitative and accurate aerosol climatology from available satellite and other measurements, thus enabling more reliable estimates of the direct and indirect aerosol forcings. The Global Aerosol Climatology Project (GACP) was established in 1998 as part of the Global Energy and Water Cycle Experiment (GEWEX). Its main objective is to analyze satellite radiance measurements and field observations to infer the global distribution of aerosols, their properties, and their seasonal and interannual variations. The overall goal is to develop advanced global aerosol climatologies for the period of satellite data and to make the aerosol climatologies broadly available through the GACP web site.

  3. The Mpi-M Aerosol Climatology (MAC)

    NASA Astrophysics Data System (ADS)

    Kinne, S.

    2014-12-01

    Monthly gridded global data-sets for aerosol optical properties (AOD, SSA and g) and for aerosol microphysical properties (CCN and IN) offer a (less complex) alternate path to include aerosol radiative effects and aerosol impacts on cloud-microphysics in global simulations. Based on merging AERONET sun-/sky-photometer data onto background maps provided by AeroCom phase 1 modeling output and AERONET sun-/the MPI-M Aerosol Climatology (MAC) version 1 was developed and applied in IPCC simulations with ECHAM and as ancillary data-set in satellite-based global data-sets. An updated version 2 of this climatology will be presented now applying central values from the more recent AeroCom phase 2 modeling and utilizing the better global coverage of trusted sun-photometer data - including statistics from the Marine Aerosol network (MAN). Applications include spatial distributions of estimates for aerosol direct and aerosol indirect radiative effects.

  4. Model-Derived Global Aerosol Climatology for MISR Analysis ("Clim-Likely" Data Set)

    Atmospheric Science Data Center

    2018-04-19

    Model-Derived Global Aerosol Climatology for MISR Analysis Multi-angle Imaging ... (MISR) monthly, global 1° x 1° "Clim-Likely" aerosol climatology, derived from 'typical-year' aerosol transport model results are available for individual 1° x 1° boxes or ...

  5. A climatology of stratospheric aerosol

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hitchman, M.H.; Mckay, M.; Trepte, C.R.

    1994-10-01

    A global climatology of stratospheric aerosol is created by combining nearly a decade (1979-1981 and 1984-1990) of contemporaneous observations from the Stratospheric Aerosol and Gas Experiment (SAGE I and II) and Stratospheric Aerosol Measurement (SAM II) instruments. One goal of this work is to provide a representative distribution of the aerosol layer for use in radiative and chemical modeling. A table of decadal average 1 micron extinction values is included, extending from the tropopause to 35 km and 80 deg S to 85 deg N, which allows estimation of surface area density. We find that the aerosol layer is distinctlymore » volcanic in nature and suggest that the decadal average is a more useful estimate of future aerosol loading than a `background` loading, which is never clearly achieved during the data record. This climatology lends insight into the general circulation of the stratosphere. Latitude - altitude sections of extinction radio at 1 micron are shown, average by decade, season, and phase of the quasi-biennial oscillation (QBO). A tropical reservoir region is diagnosed, with an `upper` and a `lower` transport regime. In the tropics above 22 km (upper regime), enhanced lofting occurs in the summer, with suppressed lofting or eddy dilution in the winter. In the extratropics within two scale heights of the tropopause (lower regime), poleward and downward transport is most robust during winter, especially in the northern hemisphere. The transport patterns persist into the subsequent equinoctial season. Ascent associated with QBO easterly shear favors detrainment in the upper regime, while relative descent and poleward spreading during QBO westerly shear favors detrainment in the lower regime. Extinction radio differences between the winter-spring and summer-fall hemispheres, and differences between the two phases of the QBO, are typically 20-50%.« less

  6. Aerosol climatology over Mexico City basin: Characterization of their optical properties

    NASA Astrophysics Data System (ADS)

    Carabali-Sandoval, Giovanni; Valdéz-Barrón, Mauro; Bonifaz-Alfonso, Roberto; Riveros-Rosas, David; Estévez, Héctor

    2015-04-01

    Climatology of aerosol optical depth (AOD), single scattering albedo (SSA) and size parameters were analyzed using a 15-year (1999-2014) data set from AErosol RObotic NETwork (AERONET) observations over Mexico City basin. Since urban air pollution is one of the biggest problems that face this megacity, many studies addressing these issues have been published. However few studies have examined the climatology of aerosol taking into account their optical properties over long-time period. Pollution problems in Mexico City have been generated by the daily activities of some 21 million people coupled with the vast amount of industry located within the city's metropolitan area. Another contributing factor is the unique geographical setting of the basin encompassing Mexico City. The basin covers approximately 5000 km2 of the Mexican Plateau at an average elevation of 2250 m above sea level (ASL) and is surrounded on three sides by mountains averaging over 3000 m ASL. In this work we present preliminary results of aerosol climatology in Mexico City.

  7. Impacts of different aerosol climatologies on the European climate during the last decades

    NASA Astrophysics Data System (ADS)

    Schultze, Markus; Rockel, Burkhardt

    2015-04-01

    As summarized in the 5th Assessment Report of the IPCC, the effects of aerosols on the Earth's energy budget are one of the largest uncertainties in a changing climate. Despite a better understanding of aerosol processes since the previous report, it remains unclear to which degree of complexity these processes need to be represented within the climate models to consider their effects in a sufficient manner. Within the nonhydrostatic regional climate model COSMO-CLM, the aerosol climatology of Tanre from 1984 is widely used to simulate the direct effect of aerosols on radiative processes. Apart from a very low spatial resolution and a missing temporal variability, this climatology is dominated by high values of Aerosol Optical Depth (AOD) over Northern Africa, caused by an overestimation of Saharan dust. To investigate the impacts of different aerosol distributions on the European climate, the Tanre aerosol climatology is replaced by the more realistic climatologies of Tegen from 1997 and AEROCOM from 2006 with constant annual cycles of AOD. In addition a control simulation without any aerosol feedbacks was performed. The simulations cover a period of 30 years from 1980 to 2010. In parts of the regions surveyed, we found a near surface cooling, which is strongly linked to AOD, and a broad mid-troposphere warming for all simulations in comparison to the control simulation. A decrease in convective precipitation is mainly caused by stabilization of stratification and by less evapotranspiration resulting from surface cooling. The horizontal differing mid-troposphere warming induces a drop in surface pressure and therefore leads to changes in circulation patterns which are still under investigation. The largest impacts of direct and semi direct aerosol effects was found in summer season. As next step, pre-calculated transient aerosol data will be used to compile an up-to-date aerosol climatology including temporal changes. One main focus of the study will be to

  8. MAC-v1: A new global aerosol climatology for climate studies

    NASA Astrophysics Data System (ADS)

    Kinne, Stefan; O'Donnel, Declan; Stier, Philip; Kloster, Silvia; Zhang, Kai; Schmidt, Hauke; Rast, Sebastian; Giorgetta, Marco; Eck, Tom F.; Stevens, Bjorn

    2013-12-01

    The Max-Planck-Institute Aerosol Climatology version 1 (MAC-v1) is introduced. It describes the optical properties of tropospheric aerosols on monthly timescales and with global coverage at a spatial resolution of 1° in latitude and longitude. By providing aerosol radiative properties for any wavelength of the solar (or shortwave) and of the terrestrial (or longwave) radiation spectrum, as needed in radiative transfer applications, this MAC-v1 data set lends itself to simplified and computationally efficient representations of tropospheric aerosol in climate studies. Estimates of aerosol radiative properties are provided for both total and anthropogenic aerosol in annual time steps from preindustrial times (i.e., starting with year 1860) well into the future (until the year 2100). Central to the aerosol climatology is the merging of monthly statistics of aerosol optical properties for current (year 2000) conditions. Hereby locally sparse but trusted high-quality data by ground-based sun-photometer networks are merged onto complete background maps defined by central data from global modeling with complex aerosol modules. This merging yields 0.13 for the global annual midvisible aerosol optical depth (AOD), with 0.07 attributed to aerosol sizes larger than 1 µm in diameter and 0.06 of attributed to aerosol sizes smaller than 1 µm in diameter. Hereby larger particles are less absorbing with a single scattering albedo (SSA) of 0.98 compared to 0.93 for smaller sizes. Simulation results of a global model are applied to prescribe the vertical distribution and to estimate anthropogenic contributions to the smaller size AOD as a function of time, with a 0.037 value for current conditions. In a demonstration application, the associated aerosol direct radiative effects are determined. For current conditions, total aerosol is estimated to reduce the combined shortwave and longwave net-flux balance at the top of the atmosphere by about -1.6 W/m2 from which -0.5 W/m2 (with

  9. A Climatology of Global Aerosol Mixtures to Support Sentinel-5P and Earthcare Mission Applications

    NASA Astrophysics Data System (ADS)

    Taylor, M.; Kazadzis, S.; Amaridis, V.; Kahn, R. A.

    2015-11-01

    Since constraining aerosol type with satellite remote sensing continues to be a challenge, we present a newly derived global climatology of aerosol mixtures to support atmospheric composition studies that are planned for Sentinel-5P and EarthCARE.The global climatology is obtained via application of iterative cluster analysis to gridded global decadal and seasonal mean values of the aerosol optical depth (AOD) of sulfate, biomass burning, mineral dust and marine aerosol as a proportion of the total AOD at 500nm output from the Goddard Chemistry Aerosol Radiation and Transport (GOCART). For both the decadal and seasonal means, the number of aerosol mixtures (clusters) identified is ≈10. Analysis of the percentage contribution of the component aerosol types to each mixture allowed development of a straightforward naming convention and taxonomy, and assignment of primary colours for the generation of true colour-mixing and easy-to-interpret maps of the spatial distribution of clusters across the global grid. To further help characterize the mixtures, aerosol robotic network (AERONET) Level 2.0 Version 2 inversion products were extracted from each cluster‟s spatial domain and used to estimate climatological values of key optical and microphysical parameters.The aerosol type climatology represents current knowledge that would be enhanced, possibly corrected, and refined by high temporal and spectral resolution, cloud-free observations produced by Sentinel-5P and EarthCARE instruments. The global decadal mean and seasonal gridded partitions comprise a preliminary reference framework and global climatology that can help inform the choice of components and mixtures in aerosol retrieval algorithms used by instruments such as TROPOMI and ATLID, and to test retrieval results.

  10. Development and Testing of the New Surface LER Climatology for OMI UV Aerosol Retrievals

    NASA Technical Reports Server (NTRS)

    Gupta, Pawan; Torres, Omar; Jethva, Hiren; Ahn, Changwoo

    2014-01-01

    Ozone Monitoring Instrument (OMI) onboard Aura satellite retrieved aerosols properties using UV part of solar spectrum. The OMI near UV aerosol algorithm (OMAERUV) is a global inversion scheme which retrieves aerosol properties both over ocean and land. The current version of the algorithm makes use of TOMS derived Lambertian Equivalent Reflectance (LER) climatology. A new monthly climatology of surface LER at 354 and 388 nm have been developed. This will replace TOMS LER (380 nm and 354nm) climatology in OMI near UV aerosol retrieval algorithm. The main objectives of this study is to produce high resolution (quarter degree) surface LER sets as compared to existing one degree TOMS surface LERs, to product instrument and wavelength consistent surface climatology. Nine years of OMI observations have been used to derive monthly climatology of surface LER. MODIS derived aerosol optical depth (AOD) have been used to make aerosol corrections on OMI wavelengths. MODIS derived BRDF adjusted reflectance product has been also used to capture seasonal changes in the surface characteristics. Finally spatial and temporal averaging techniques have been used to fill the gaps around the globes, especially in the regions with consistent cloud cover such as Amazon. After implementation of new surface data in the research version of algorithm, comparisons of AOD and single scattering albedo (SSA) have been performed over global AERONET sites for year 2007. Preliminary results shows improvements in AOD retrievals globally but more significance improvement were observed over desert and bright locations. We will present methodology of deriving surface data sets and will discuss the observed changes in retrieved aerosol properties with respect to reference AERONET measurements.

  11. Climatological Aspects of the Optical Properties of Fine/Coarse Mode Aerosol Mixtures

    NASA Technical Reports Server (NTRS)

    Eck, T. F.; Holben, B. N.; Sinyuk, A.; Pinker, R. T.; Goloub, P.; Chen, H.; Chatenet, B.; Li, Z.; Singh, R. P.; Tripathi, S.N.; hide

    2010-01-01

    Aerosol mixtures composed of coarse mode desert dust combined with fine mode combustion generated aerosols (from fossil fuel and biomass burning sources) were investigated at three locations that are in and/or downwind of major global aerosol emission source regions. Multiyear monitoring data at Aerosol Robotic Network sites in Beijing (central eastern China), Kanpur (Indo-Gangetic Plain, northern India), and Ilorin (Nigeria, Sudanian zone of West Africa) were utilized to study the climatological characteristics of aerosol optical properties. Multiyear climatological averages of spectral single scattering albedo (SSA) versus fine mode fraction (FMF) of aerosol optical depth at 675 nm at all three sites exhibited relatively linear trends up to 50% FMF. This suggests the possibility that external linear mixing of both fine and coarse mode components (weighted by FMF) dominates the SSA variation, where the SSA of each component remains relatively constant for this range of FMF only. However, it is likely that a combination of other factors is also involved in determining the dynamics of SSA as a function of FMF, such as fine mode particles adhering to coarse mode dust. The spectral variation of the climatological averaged aerosol absorption optical depth (AAOD) was nearly linear in logarithmic coordinates over the wavelength range of 440-870 nm for both the Kanpur and Ilorin sites. However, at two sites in China (Beijing and Xianghe), a distinct nonlinearity in spectral AAOD in logarithmic space was observed, suggesting the possibility of anomalously strong absorption in coarse mode aerosols increasing the 870 nm AAOD.

  12. Climatology and Characteristics of Aerosol Optical Properties in the Arctic

    NASA Astrophysics Data System (ADS)

    Schmeisser, Lauren; Ogren, John; Backman, John; Asmi, Eija; Andrews, Elisabeth; Jefferson, Anne; Bergin, Michael; Tunved, Peter; Sharma, Sangeeta; Starkweather, Sandra

    2016-04-01

    Within the Arctic, climate forcers like atmospheric aerosols are important contributors to the observed warming and environmental changes in the region. Quantifying the forcing by aerosols in the Arctic is especially difficult, given short aerosol lifetimes, annual variability in illumination and surface albedo, stratified atmospheric conditions, complex feedbacks, and long-range aerosol transport. However, in-situ surface measurements of Arctic aerosol optical properties can be used to constrain variability of light scattering and absorption, identify potential particle sources, and help evaluate the resulting forcing. Data from six WMO Global Atmosphere Watch stations are presented: Alert, Canada (ALT); Barrow, Alaska (BRW); Pallas, Finland (PAL); Summit, Greenland (SUM); Tiksi, Russia (TIK); and Zeppelin Mountain, Norway (ZEP). These sites contribute to the International Arctic System for Observing the Atmosphere (IASOA), which facilitates Arctic-wide data collection and analysis. Climatologies of aerosol optical properties from each station show differences in magnitude and variability of observed parameters. For example, most stations (ALT, BRW, SUM, TIK, ZEP) experience maximum scattering in winter/spring, while PAL exhibits maximum scattering in the summer. The observed range in scattering across these sites is large (almost an order of magnitude) - SUM has the lowest annual median scattering at 0.82 Mm-1 while BRW has the highest at 6.9 Mm-1. A closer look at systematic variability between optical properties at each station, as well as site back trajectories, suggest differences in aerosol processes, sources and transport. The development of consistent climatologies and additional analyses like the ones presented here can help provide a better understanding of trans-Arctic aerosol variability, which can be an asset for improving aerosol models in this unique and remote region.

  13. Aerosol climatology using a tunable spectral variability cloud screening of AERONET data

    NASA Technical Reports Server (NTRS)

    Kaufman, Yoram J.; Gobbi, Gian Paolo; Koren, Ilan

    2005-01-01

    Can cloud screening of an aerosol data set, affect the aerosol optical thickness (AOT) climatology? Aerosols, humidity and clouds are correlated. Therefore, rigorous cloud screening can systematically bias towards less cloudy conditions, underestimating the average AOT. Here, using AERONET data we show that systematic rejection of variable atmospheric optical conditions can generate such bias in the average AOT. Therefore we recommend (1) to introduce more powerful spectral variability cloud screening and (2) to change the philosophy behind present aerosol climatologies: Instead of systematically rejecting all cloud contaminations, we suggest to intentionally allow the presence of cloud contamination, estimate the statistical impact of the contamination and correct for it. The analysis, applied to 10 AERONET stations with approx. 4 years of data, shows almost no change for Rome (Italy), but up to a change in AOT of 0.12 in Beijing (PRC). Similar technique may be explored for satellite analysis, e.g. MODIS.

  14. Validation of Long-Term Global Aerosol Climatology Project Optical Thickness Retrievals Using AERONET and MODIS Data

    NASA Technical Reports Server (NTRS)

    Geogdzhayev, Igor V.; Mishchenko, Michael I.

    2015-01-01

    A comprehensive set of monthly mean aerosol optical thickness (AOT) data from coastal and island AErosol RObotic NETwork (AERONET) stations is used to evaluate Global Aerosol Climatology Project (GACP) retrievals for the period 1995-2009 during which contemporaneous GACP and AERONET data were available. To put the GACP performance in broader perspective, we also compare AERONET and MODerate resolution Imaging Spectroradiometer (MODIS) Aqua level-2 data for 2003-2009 using the same methodology. We find that a large mismatch in geographic coverage exists between the satellite and ground-based datasets, with very limited AERONET coverage of open-ocean areas. This is especially true of GACP because of the smaller number of AERONET stations at the early stages of the network development. Monthly mean AOTs from the two over-the-ocean satellite datasets are well-correlated with the ground-based values, the correlation coefficients being 0.81-0.85 for GACP and 0.74-0.79 for MODIS. Regression analyses demonstrate that the GACP mean AOTs are approximately 17%-27% lower than the AERONET values on average, while the MODIS mean AOTs are 5%-25% higher. The regression coefficients are highly dependent on the weighting assumptions (e.g., on the measure of aerosol variability) as well as on the set of AERONET stations used for comparison. Comparison of over-the-land and over-the-ocean MODIS monthly mean AOTs in the vicinity of coastal AERONET stations reveals a significant bias. This may indicate that aerosol amounts in coastal locations can differ significantly from those in adjacent open-ocean areas. Furthermore, the color of coastal waters and peculiarities of coastline meteorological conditions may introduce biases in the GACP AOT retrievals. We conclude that the GACP and MODIS over-the-ocean retrieval algorithms show similar ranges of discrepancy when compared to available coastal and island AERONET stations. The factors mentioned above may limit the performance of the

  15. Evaluation of spatio-temporal variability of Hamburg Aerosol Climatology against aerosol datasets from MODIS and CALIOP

    NASA Astrophysics Data System (ADS)

    Pappas, V.; Hatzianastassiou, N.; Papadimas, C.; Matsoukas, C.; Kinne, S.; Vardavas, I.

    2013-08-01

    The new global aerosol climatology named HAC (Hamburg Aerosol Climatology) is compared against MODIS (Collection 5, 2000-2007) and CALIOP (Level 2-version 3, 2006-2011) retrievals. The comparison of aerosol optical depth (AOD) from HAC against MODIS shows larger HAC AOD values over regions with higher aerosol loads and smaller HAC AOD values than MODIS for regions with lower loads. The HAC data are found to be more reliable over land and for low AOD values. The largest differences between HAC and MODIS occur from March to August for the Northern Hemisphere and from September to February for the Southern Hemisphere. In addition, both the spectral variability and vertical distribution of the HAC AOD are examined at selected AERONET (1998-2007) sites, representative of main aerosol types (pollutants, sea salt, biomass and dust). Based on comparisons against spectral AOD values from AERONET, the mean absolute percentage error in HAC AOD data is 25% at ultraviolet wavelengths (400 nm), 6-12% at visible and 18% at near-infrared (1000 nm). For the same AERONET sites, the HAC AOD vertical distribution is compared against CALIOP space lidar data. On a daily average basis, HAD AOD is less by 9% in the lowest 3 km than CALIOP values, especially for sites with biomass burning smoke, desert dust and sea salt spray. Above the boundary layer, the HAC AOD vertical distribution is reliable.

  16. Steps Toward an EOS-Era Aerosol Air Mass Type Climatology

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.

    2012-01-01

    We still have a way to go to develop a global climatology of aerosol type from the EOS-era satellite data record that currently spans more than 12 years of observations. We have demonstrated the ability to retrieve aerosol type regionally, providing a classification based on the combined constraints on particle size, shape, and single-scattering albedo (SSA) from the MISR instrument. Under good but not necessarily ideal conditions, the MISR data can distinguish three-to-five size bins, two-to-four bins in SSA, and spherical vs. non-spherical particles. However, retrieval sensitivity varies enormously with scene conditions. So, for example, there is less information about aerosol type when the mid-visible aerosol optical depth (AOD) is less that about 0.15 or 0.2.

  17. Evaluation of spatio-temporal variability of Hamburg Aerosol Climatology against aerosol datasets from MODIS and CALIOP

    NASA Astrophysics Data System (ADS)

    Pappas, V.; Hatzianastassiou, N.; Papadimas, C.; Matsoukas, C.; Kinne, S.; Vardavas, I.

    2013-02-01

    The new global aerosol climatology named HAC (Hamburg Aerosol Climatology) is compared against MODIS (MODerate resolution Imaging Spectroradiometer, Collection 5, 2000-2007) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization, Level 2-Version 3, 2006-2011) retrievals. The HAC aerosol optical depth (AOD) values are larger than MODIS in heavy aerosol load conditions (over land) and lower over oceans. Agreement between HAC and MODIS is better over land and for low AOD. Hemispherically, HAC has 16-17% smaller AOD values than MODIS. The discrepancy is slightly larger for the Southern Hemisphere (SH) than for the Northern Hemisphere (NH). Seasonally, the largest absolute differences are from March to August for NH and from September to February for SH. The spectral variability of HAC AOD is also evaluated against AERONET (1998-2007) data for sites representative of main aerosol types (pollutants, sea-salt, biomass and dust). The HAC has a stronger spectral dependence of AOD in the UV wavelengths, compared to AERONET and MODIS. For visible and near-infrared wavelengths, the spectral dependence is similar to AERONET. For specific sites, HAC AOD vertical distribution is compared to CALIOP data by looking at the fraction of columnar AOD at each altitude. The comparison suggests that HAC exhibits a smaller fraction of columnar AOD in the lowest 2-3 km than CALIOP, especially for sites with biomass burning smoke, desert dust and sea salt spray. For the region of the greater Mediterranean basin, the mean profile of HAC AOD is in very good agreement with CALIOP. The HAC AOD is very useful for distinguishing between natural and anthropogenic aerosols and provides high spectral resolution and vertically resolved information.

  18. an aerosol climatology optical properties and its associated direct radiative forcing

    NASA Astrophysics Data System (ADS)

    Kinne, Stefan

    2010-05-01

    Aerosol particles are quite complex in nature. Aerosol impacts on the distribution of radiative energy and on cloud microphysics have been debated climate impact issues. Here, a new aerosol-climatology is presented, combining the consistency and completeness of global modelling with quality data by ground-monitoring. It provides global monthly maps for spectral aerosol optical properties and for concentrations of CCN and IN. Based on the optical properties the aerosol direct forcing is determined. And with environmental data for clouds and estimates on the anthropogenic fraction from emission experiments with global modelling even the climate relevant aerosol direct forcing at the top of the atmosphere (ToA) is determined. This value is rather small near -0.2W/m2 with limited uncertainty estimated at (+/-0.3) due to uncertainties in aerosol absorption and underlying surface conditions or clouds.

  19. Progress Toward a Global, EOS-Era Aerosol Air Mass Type Climatology

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.

    2012-01-01

    The MISR and MODIS instruments aboard the NASA Earth Observing System's Terra Satellite have been collecting data containing information about the state of Earth's atmosphere and surface for over eleven years. Data from these instruments have been used to develop a global, monthly climatology of aerosol amount that is widely used as a constraint on climate models, including those used for the 2007 IPCC assessment report. The next frontier in assessing aerosol radiative forcing of climate is aerosol type, and in particular, the absorption properties of major aerosol air masses. This presentation will focus on the prospects for constraining aerosol type globally, and the steps we are taking to apply a combination of satellite and suborbital data to this challenge.

  20. Climatology of Aerosol Optical Properties in Southern Africa

    NASA Technical Reports Server (NTRS)

    Queface, Antonio J.; Piketh, Stuart J.; Eck, Thomas F.; Tsay, Si-Chee

    2011-01-01

    A thorough regionally dependent understanding of optical properties of aerosols and their spatial and temporal distribution is required before we can accurately evaluate aerosol effects in the climate system. Long term measurements of aerosol optical depth, Angstrom exponent and retrieved single scattering albedo and size distribution, were analyzed and compiled into an aerosol optical properties climatology for southern Africa. Monitoring of aerosol parameters have been made by the AERONET program since the middle of the last decade in southern Africa. This valuable information provided an opportunity for understanding how aerosols of different types influence the regional radiation budget. Two long term sites, Mongu in Zambia and Skukuza in South Africa formed the core sources of data in this study. Results show that seasonal variation of aerosol optical thicknesses at 500 nm in southern Africa are characterized by low seasonal multi-month mean values (0.11 to 0.17) from December to May, medium values (0.20 to 0.27) between June and August, and high to very high values (0.30 to 0.46) during September to November. The spatial distribution of aerosol loadings shows that the north has high magnitudes than the south in the biomass burning season and the opposite in none biomass burning season. From the present aerosol data, no long term discernable trends are observable in aerosol concentrations in this region. This study also reveals that biomass burning aerosols contribute the bulk of the aerosol loading in August-October. Therefore if biomass burning could be controlled, southern Africa will experience a significant reduction in total atmospheric aerosol loading. In addition to that, aerosol volume size distribution is characterized by low concentrations in the non biomass burning period and well balanced particle size contributions of both coarse and fine modes. In contrast high concentrations are characteristic of biomass burning period, combined with

  1. Steps Toward an EOS-Era Aerosol Type Climatology

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.

    2012-01-01

    We still have a way to go to develop a global climatology of aerosol type from the EOS-era satellite data record that currently spans more than 12 years of observations. We have demonstrated the ability to retrieve aerosol type regionally, providing a classification based on the combined constraints on particle size, shape, and single-scattering albedo (SSA) from the MISR instrument. Under good but not necessarily ideal conditions, the MISR data can distinguish three-to-five size bins, two-to-four bins in SSA, and spherical vs. non-spherical particles. However, retrieval sensitivity varies enormously with scene conditions. So, for example, there is less information about aerosol type when the mid-visible aerosol optical depth (AOD) is less that about 0.15 or 0.2, or when the range of scattering angles observed is reduced by solar geometry, even though the quality of the AOD retrieval itself is much less sensitive to these factors. This presentation will review a series of studies aimed at assessing the capabilities, as well as the limitations, of MISR aerosol type retrievals involving wildfire smoke, desert dust, volcanic ash, and urban pollution, in specific cases where suborbital validation data are available. A synthesis of results, planned upgrades to the MISR Standard aerosol algorithm to improve aerosol type retrievals, and steps toward the development of an aerosol type quality flag for the Standard product, will also be covered.

  2. Aerosol climatology: on the discrimination of aerosol types over four AERONET sites

    NASA Astrophysics Data System (ADS)

    Kaskaoutis, D. G.; Kambezidis, H. D.; Hatzianastassiou, N.; Kosmopoulos, P. G.; Badarinath, K. V. S.

    2007-05-01

    Aerosols have a significant regional and global effect on climate, which is about equal in magnitude but opposite in sign to that of greenhouse gases. Nevertheless, the aerosol climatic effect changes strongly with space and time because of the large variability of aerosol physical and optical properties, which is due to the variety of their sources, which are natural, and anthropogenic, and their dependence on the prevailing meteorological and atmospheric conditions. Characterization of aerosol properties is of major importance for the assessment of their role for climate. In the present study, 3-year AErosol RObotic NETwork (AERONET) data from ground-based sunphotometer measurements are used to establish climatologies of aerosol optical depth (AOD) and Ångström exponent α in several key locations of the world, characteristic of different atmospheric environments. Using daily mean values of AOD at 500 nm (AOD500) and Ångström exponent at the pair of wavelengths 440 and 870 nm (α 440-870), a discrimination of the different aerosol types occurring in each location is achieved. For this discrimination, appropriate thresholds for AOD500 and α 440-870 are applied. The discrimination of aerosol types in each location is made on an annual and seasonal basis. It is shown that a single aerosol type in a given location can exist only under specific conditions (e.g. intense forest fires or dust outbreaks), while the presence of well-mixed aerosols is the accustomed situation. Background clean aerosol conditions (AOD500<0.06) are mostly found over remote oceanic surfaces occurring on average in ~56.7% of total cases, while this situation is quite rare over land (occurrence of 3.8-13.7%). Our analysis indicates that these percentages change significantly from season to season. The spectral dependence of AOD exhibits large differences between the examined locations, while it exhibits a strong annual cycle.

  3. Aerosol retrieval experiments in the ESA Aerosol_cci project

    NASA Astrophysics Data System (ADS)

    Holzer-Popp, T.; de Leeuw, G.; Martynenko, D.; Klüser, L.; Bevan, S.; Davies, W.; Ducos, F.; Deuzé, J. L.; Graigner, R. G.; Heckel, A.; von Hoyningen-Hüne, W.; Kolmonen, P.; Litvinov, P.; North, P.; Poulsen, C. A.; Ramon, D.; Siddans, R.; Sogacheva, L.; Tanre, D.; Thomas, G. E.; Vountas, M.; Descloitres, J.; Griesfeller, J.; Kinne, S.; Schulz, M.; Pinnock, S.

    2013-03-01

    Within the ESA Climate Change Initiative (CCI) project Aerosol_cci (2010-2013) algorithms for the production of long-term total column aerosol optical depth (AOD) datasets from European Earth Observation sensors are developed. Starting with eight existing pre-cursor algorithms three analysis steps are conducted to improve and qualify the algorithms: (1) a series of experiments applied to one month of global data to understand several major sensitivities to assumptions needed due to the ill-posed nature of the underlying inversion problem, (2) a round robin exercise of "best" versions of each of these algorithms (defined using the step 1 outcome) applied to four months of global data to identify mature algorithms, and (3) a comprehensive validation exercise applied to one complete year of global data produced by the algorithms selected as mature based on the round robin exercise. The algorithms tested included four using AATSR, three using MERIS and one using PARASOL. This paper summarizes the first step. Three experiments were conducted to assess the potential impact of major assumptions in the various aerosol retrieval algorithms. In the first experiment a common set of four aerosol components was used to provide all algorithms with the same assumptions. The second experiment introduced an aerosol property climatology, derived from a combination of model and sun photometer observations, as a priori information in the retrievals on the occurrence of the common aerosol components and their mixing ratios. The third experiment assessed the impact of using a common nadir cloud mask for AATSR and MERIS algorithms in order to characterize the sensitivity to remaining cloud contamination in the retrievals against the baseline dataset versions. The impact of the algorithm changes was assessed for one month (September 2008) of data qualitatively by visible analysis of monthly mean AOD maps and quantitatively by comparing global daily gridded satellite data against daily

  4. Towards a Global Aerosol Climatology: Preliminary Trends in Tropospheric Aerosol Amounts and Corresponding Impact on Radiative Forcing between 1950 and 1990

    NASA Technical Reports Server (NTRS)

    Tegen, Ina; Koch, Dorothy; Lacis, Andrew A.; Sato, Makiko

    1999-01-01

    A global aerosol climatology is needed in the study of decadal temperature change due to natural and anthropogenic forcing of global climate change. A preliminary aerosol climatology has been developed from global transport models for a mixture of sulfate and carbonaceous aerosols from fossil fuel burning, including also contributions from other major aerosol types such as soil dust and sea salt. The aerosol distributions change for the period of 1950 to 1990 due to changes in emissions of SO2 and carbon particles from fossil fuel burning. The optical thickness of fossil fuel derived aerosols increased by nearly a factor of 3 during this period, with particularly strong increase in eastern Asia over the whole time period. In countries where environmental laws came into effect since the early 1980s (e.g. US and western Europe), emissions and consequently aerosol optical thicknesses did not increase considerably after 1980, resulting in a shift in the global distribution pattern over this period. In addition to the optical thickness, aerosol single scattering albedos may have changed during this period due to different trends in absorbing black carbon and reflecting sulfate aerosols. However, due to the uncertainties in the emission trends, this change cannot be determined with any confidence. Radiative forcing of this aerosol distribution is calculated for several scenarios, resulting in a wide range of uncertainties for top-of-atmosphere (TOA) forcings. Uncertainties in the contribution of the strongly absorbing black carbon aerosol leads to a range in TOA forcings of ca. -0.5 to + 0.1 Wm (exp. -2), while the change in aerosol distributions between 1950 to 1990 leads to a change of -0.1 to -0.3 Wm (exp. -2), for fossil fuel derived aerosol with a "moderate" contribution of black carbon aerosol.

  5. Aerosol retrieval experiments in the ESA Aerosol_cci project

    NASA Astrophysics Data System (ADS)

    Holzer-Popp, T.; de Leeuw, G.; Griesfeller, J.; Martynenko, D.; Klüser, L.; Bevan, S.; Davies, W.; Ducos, F.; Deuzé, J. L.; Graigner, R. G.; Heckel, A.; von Hoyningen-Hüne, W.; Kolmonen, P.; Litvinov, P.; North, P.; Poulsen, C. A.; Ramon, D.; Siddans, R.; Sogacheva, L.; Tanre, D.; Thomas, G. E.; Vountas, M.; Descloitres, J.; Griesfeller, J.; Kinne, S.; Schulz, M.; Pinnock, S.

    2013-08-01

    Within the ESA Climate Change Initiative (CCI) project Aerosol_cci (2010-2013), algorithms for the production of long-term total column aerosol optical depth (AOD) datasets from European Earth Observation sensors are developed. Starting with eight existing pre-cursor algorithms three analysis steps are conducted to improve and qualify the algorithms: (1) a series of experiments applied to one month of global data to understand several major sensitivities to assumptions needed due to the ill-posed nature of the underlying inversion problem, (2) a round robin exercise of "best" versions of each of these algorithms (defined using the step 1 outcome) applied to four months of global data to identify mature algorithms, and (3) a comprehensive validation exercise applied to one complete year of global data produced by the algorithms selected as mature based on the round robin exercise. The algorithms tested included four using AATSR, three using MERIS and one using PARASOL. This paper summarizes the first step. Three experiments were conducted to assess the potential impact of major assumptions in the various aerosol retrieval algorithms. In the first experiment a common set of four aerosol components was used to provide all algorithms with the same assumptions. The second experiment introduced an aerosol property climatology, derived from a combination of model and sun photometer observations, as a priori information in the retrievals on the occurrence of the common aerosol components. The third experiment assessed the impact of using a common nadir cloud mask for AATSR and MERIS algorithms in order to characterize the sensitivity to remaining cloud contamination in the retrievals against the baseline dataset versions. The impact of the algorithm changes was assessed for one month (September 2008) of data: qualitatively by inspection of monthly mean AOD maps and quantitatively by comparing daily gridded satellite data against daily averaged AERONET sun photometer

  6. Toward a Combined SAGE II-HALOE Aerosol Climatology: An Evaluation of HALOE Version 19 Stratospheric Aerosol Extinction Coefficient Observations

    NASA Technical Reports Server (NTRS)

    Thomason, L. W.

    2012-01-01

    Herein, the Halogen Occultation Experiment (HALOE) aerosol extinction coefficient data is evaluated in the low aerosol loading period after 1996 as the first necessary step in a process that will eventually allow the production of a combined HALOE/SAGE II (Stratospheric Aerosol and Gas Experiment) aerosol climatology of derived aerosol products including surface area density. Based on these analyses, it is demonstrated that HALOE's 3.46 microns is of good quality above 19 km and suitable for scientific applications above that altitude. However, it is increasingly suspect at lower altitudes and should not be used below 17 km under any circumstances after 1996. The 3.40 microns is biased by about 10% throughout the lower stratosphere due to the failure to clear NO2 but otherwise appears to be a high quality product down to 15 km. The 2.45 and 5.26 micron aerosol extinction coefficient measurements are clearly biased and should not be used for scientific applications after the most intense parts of the Pinatubo period. Many of the issues in the aerosol data appear to be related to either the failure to clear some interfering gas species or doing so poorly. For instance, it is clear that the 3.40micronaerosol extinction coefficient measurements can be improved through the inclusion of an NO2 correction and could, in fact, end up as the highest quality overall HALOE aerosol extinction coefficient measurement. It also appears that the 2.45 and 5.26 micron channels may be improved by updating the Upper Atmosphere Pilot Database which is used as a resource for the removal of gas species otherwise not available from direct HALOE measurements. Finally, a simple model to demonstrate the promise of mixed visible/infrared aerosol extinction coefficient ensembles for the retrieval of bulk aerosol properties demonstrates that a combined HALOE/SAGE II aerosol climatology is feasible and may represent a substantial improvement over independently derived data sets.

  7. Direct and semi-direct effects of aerosol climatologies on long-term climate simulations over Europe

    NASA Astrophysics Data System (ADS)

    Schultze, Markus; Rockel, Burkhardt

    2017-08-01

    This study compares the direct and semi-direct aerosol effects of different annual cycles of tropospheric aerosol loads for Europe from 1950 to 2009 using the regional climate model COSMO-CLM, which is laterally forced by reanalysis data and run using prescribed, climatological aerosol optical properties. These properties differ with respect to the analysis strategy and the time window, and are then used for the same multi-decadal period. Five simulations with different aerosol loads and one control simulation without any tropospheric aerosols are integrated and compared. Two common limitations of our simulation strategy, to fully assess direct and semi-direct aerosol effects, are the applied observed sea surface temperatures and sea ice conditions, and the lack of short-term variations in the aerosol load. Nevertheless, the impact of different aerosol climatologies on common regional climate model simulations can be assessed. The results of all aerosol-including simulations show a distinct reduction in solar irradiance at the surface compared with that in the control simulation. This reduction is strongest in the summer season and is balanced primarily by a weakening of turbulent heat fluxes and to a lesser extent by a decrease in longwave emissions. Consequently, the seasonal mean surface cooling is modest. The temperature profile responses are characterized by a shallow near-surface cooling and a dominant warming up to the mid-troposphere caused by aerosol absorption. The resulting stabilization of stratification leads to reduced cloud cover and less precipitation. A decrease in cloud water and ice content over Central Europe in summer possibly reinforce aerosol absorption and thus strengthen the vertical warming. The resulting radiative forcings are positive. The robustness of the results was demonstrated by performing a simulation with very strong aerosol forcing, which lead to qualitatively similar results. A distinct added value over the default aerosol

  8. A global space-based stratospheric aerosol climatology: 1979-2016

    NASA Astrophysics Data System (ADS)

    Thomason, Larry W.; Ernest, Nicholas; Millán, Luis; Rieger, Landon; Bourassa, Adam; Vernier, Jean-Paul; Manney, Gloria; Luo, Beiping; Arfeuille, Florian; Peter, Thomas

    2018-03-01

    We describe the construction of a continuous 38-year record of stratospheric aerosol optical properties. The Global Space-based Stratospheric Aerosol Climatology, or GloSSAC, provided the input data to the construction of the Climate Model Intercomparison Project stratospheric aerosol forcing data set (1979-2014) and we have extended it through 2016 following an identical process. GloSSAC focuses on the Stratospheric Aerosol and Gas Experiment (SAGE) series of instruments through mid-2005, and on the Optical Spectrograph and InfraRed Imager System (OSIRIS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data thereafter. We also use data from other space instruments and from ground-based, air, and balloon borne instruments to fill in key gaps in the data set. The end result is a global and gap-free data set focused on aerosol extinction coefficient at 525 and 1020 nm and other parameters on an "as available" basis. For the primary data sets, we developed a new method for filling the post-Pinatubo eruption data gap for 1991-1993 based on data from the Cryogenic Limb Array Etalon Spectrometer. In addition, we developed a new method for populating wintertime high latitudes during the SAGE period employing a latitude-equivalent latitude conversion process that greatly improves the depiction of aerosol at high latitudes compared to earlier similar efforts. We report data in the troposphere only when and where it is available. This is primarily during the SAGE II period except for the most enhanced part of the Pinatubo period. It is likely that the upper troposphere during Pinatubo was greatly enhanced over non-volcanic periods and that domain remains substantially under-characterized. We note that aerosol levels during the OSIRIS/CALIPSO period in the lower stratosphere at mid- and high latitudes is routinely higher than what we observed during the SAGE II period. While this period had nearly continuous low-level volcanic activity, it

  9. Downward solar global irradiance at the surface in São Paulo city—The climatological effects of aerosol and clouds

    NASA Astrophysics Data System (ADS)

    Yamasoe, M. A.; do Rosário, N. M. E.; Barros, K. M.

    2017-01-01

    We analyzed the variability of downward solar irradiance reaching the surface at São Paulo city, Brazil, and estimated the climatological aerosol and cloud radiative effects. Eleven years of irradiance were analyzed, from 2005 to 2015. To distinguish the aerosol from the cloud effect, the radiative transfer code LibRadtran was used to calculate downward solar irradiance. Two runs were performed, one considering only ozone and water vapor daily variability, with AOD set to zero and the second allowing the three variables to change, according to mean climatological values. The difference of the 24 h mean irradiance calculated with and without aerosol resulted in the shortwave aerosol direct radiative effect, while the difference between the measured and calculated, including the aerosol, represented the cloud effect. Results showed that, climatologically, clouds can be 4 times more effective than aerosols. The cloud shortwave radiative effect presented a maximum reduction of about -170 W m-2 in January and a minimum in July, of -37 W m-2. The aerosol direct radiative effect was maximum in spring, when the transport of smoke from the Amazon and central parts of South America is frequent toward São Paulo. Around mid-September, the 24 h radiative effect due to aerosol only was estimated to be -50 W m-2. Throughout the rest of the year, the mean aerosol effect was around -20 W m-2 and was attributed to local urban sources. The effect of the cloud fraction on the cloud modification factor, defined as the ratio of all-sky irradiation to cloudless sky irradiation, showed dependence on the cloud height. Low clouds presented the highest impact while the presence of high clouds only almost did not affect solar transmittance, even in overcast conditions.

  10. Long-term aerosol climatology over Indo-Gangetic Plain: Trend, prediction and potential source fields

    NASA Astrophysics Data System (ADS)

    Kumar, M.; Parmar, K. S.; Kumar, D. B.; Mhawish, A.; Broday, D. M.; Mall, R. K.; Banerjee, T.

    2018-05-01

    Long-term aerosol climatology is derived using Terra MODIS (Collection 6) enhanced Deep Blue (DB) AOD retrieval algorithm to investigate decadal trend (2006-2015) in columnar aerosol loading, future scenarios and potential source fields over the Indo-Gangetic Plain (IGP), South Asia. Satellite based aerosol climatology was analyzed in two contexts: for the entire IGP considering area weighted mean AOD and for nine individual stations located at upper (Karachi, Multan, Lahore), central (Delhi, Kanpur, Varanasi, Patna) and lower IGP (Kolkata, Dhaka). A comparatively high aerosol loading (AOD: 0.50 ± 0.25) was evident over IGP with a statistically insignificant increasing trend of 0.002 year-1. Analysis highlights the existing spatial and temporal gradients in aerosol loading with stations over central IGP like Varanasi (decadal mean AOD±SD; 0.67 ± 0.28) and Patna (0.65 ± 0.30) exhibit the highest AOD, followed by stations over lower IGP (Kolkata: 0.58 ± 0.21; Dhaka: 0.60 ± 0.24), with a statistically significant increasing trend (0.0174-0.0206 year-1). In contrast, stations over upper IGP reveal a comparatively low aerosol loading, having an insignificant increasing trend. Variation in AOD across IGP is found to be mainly influenced by seasonality and topography. A distinct "aerosol pool" region over eastern part of Ganges plain is identified, where meteorology, topography, and aerosol sources favor the persistence of airborne particulates. A strong seasonality in aerosol loading and types is also witnessed, with high AOD and dominance of fine particulates over central to lower IGP, especially during post-monsoon and winter. The time series analyses by autoregressive integrated moving average (ARIMA) indicate contrasting patterns in randomness of AOD over individual stations with better performance especially over central IGP. Concentration weighted trajectory analyses identify the crucial contributions of western dry regions and partial contributions from

  11. An Emerging Global Aerosol Climatology from the MODIS Satellite Sensors

    NASA Technical Reports Server (NTRS)

    Remer, Lorraine A.; Kleidman, Richard G.; Levy, Robert C.; Kaufman, Yoram J.; Tanre, Didier; Mattoo, Shana; Martins, J. Vandelei; Ichoku, Charles; Koren, Ilan; Hongbin, Yu; hide

    2008-01-01

    The recently released Collection 5 MODIS aerosol products provide a consistent record of the Earth's aerosol system. Comparison with ground-based AERONET observations of aerosol optical depth (AOD) we find that Collection 5 MODIS aerosol products estimate AOD to within expected accuracy more than 60% of the time over ocean and more than 72% of the time over land. This is similar to previous results for ocean, and better than the previous results for land. However, the new Collection introduces a 0.01 5 offset between the Terra and Aqua global mean AOD over ocean, where none existed previously. Aqua conforms to previous values and expectations while Terra is high. The cause of the offset is unknown, but changes to calibration are a possible explanation. We focus the climatological analysis on the better understood Aqua retrievals. We find that global mean AOD at 550 nm over oceans is 0.13 and over land 0.19. AOD in situations with 80% cloud fraction are twice the global mean values, although such situations occur only 2% of the time over ocean and less than 1% of the time over land. There is no drastic change in aerosol particle size associated with these very cloudy situations. Regionally, aerosol amounts vary from polluted areas such as East Asia and India, to the cleanest regions such as Australia and the northern continents. In almost all oceans fine mode aerosol dominates over dust, except in the tropical Atlantic downwind of the Sahara and in some months the Arabian Sea.

  12. A global, space-based stratospheric aerosol climatology: 1979 to 2014

    NASA Astrophysics Data System (ADS)

    Thomason, L. W.; Vernier, J. P.; Bourassa, A. E.; Millan, L.; Manney, G. L.

    2016-12-01

    Herein, we report on a global space-based stratospheric aerosol climatology (GloSSAC) that has been developed to support Coupled Model Intercomparison Project Phase 6 (CMIP6) (REF to CMIP6 and ETH work). GloSSAC is most closely related to the ASAP[SPARC, 2006] and CCMI data sets and follows a similar approach used to produce those data sets. It is primarily built using space-based measurements by a number of instruments including the SAGE series, OSIRIS, CALIPSO, CLAES and HALOE. The data set is presented as monthly depictions for 80S to 80N and from at least the tropopause to 40 km. The data set consists primarily of measurements by the instruments at their native wavelength and measurement type (e.g., extinction coefficient). However, every bin in these monthly grids receives measured or indirectly inferred values for aerosol extinction coefficient at 525 and 1020 nm. Generally, bins where no data are available are filled via simple linear interpolation in time only. The exceptions are in the SAGE I/II gap from 1982 to 1984 where data from SAM II and ground-based and airborne lidar data sets are used to span the 3 years between the end of the SAGE I mission in November 1981 and the beginning of the SAGE II mission in October 1984. Ground-based lidar also supplements space-based data in the months following the Pinatubo eruption when much of the lower stratosphere is too optically opaque for occultation measurements. This data set includes total aerosol surface area density and volume estimates based on Thomason et al.[2008] though these should be interpreted as bounding values (low and high) rather than functional aerosol parameters that are generally produced from this and predecessor data sets by other parties. Unlike previous versions of this data set, GloSSAC has been permanently archived at NASA's Atmospheric Science Data Center and a digital object identifier (doi) for GloSSAC is available. SPARC (2006), Assessment of Stratospheric Aerosol Properties (ASAP

  13. Towards climatological study on the characteristics of aerosols in Central Africa and Mediterranean sites

    NASA Astrophysics Data System (ADS)

    Benkhalifa, Jamel; Chaabane, Mabrouk

    2016-02-01

    The atmosphere contains molecules, clouds and aerosols that are sub-millimeter particles having a large variability in size, shape, chemical composition, lifetime and contents. The aerosols concentration depends greatly on the geographical situation, meteorological and environmental conditions, which makes aerosol climatology difficult to assess. Setting up a solar photometer (automatic, autonomous and portable instrument) on a given site allows carrying out the necessary measurements for aerosol characterization. The particle microphysical and optical properties are obtained from photometric measurements. The objective of this study is to analyze the spatial variability of aerosol optical thickness (AOT) in several Mediterranean regions and Central Africa, we considered a set of simultaneous data in the AErosol RObotic NETwork (AERONET) from six sites, two of which are located in Central Africa (Banizoumbou and Zinder Airport) and the rest are Mediterranean sites (Barcelona, Malaga, Lampedusa, and Forth Crete). The results have shown that the physical properties of aerosols are closely linked to the climate nature of the studied site. The optical thickness, single scattering albedo and aerosols size distribution can be due to the aging of the dust aerosol as they are transported over the Mediterranean basin.

  14. An aerosol optical depth climatology for NOAA's national surface radiation budget network (SURFRAD)

    NASA Astrophysics Data System (ADS)

    Augustine, John A.; Hodges, Gary B.; Dutton, Ellsworth G.; Michalsky, Joseph J.; Cornwall, Christopher R.

    2008-06-01

    A series of algorithms developed to process spectral solar measurements for aerosol optical depth (AOD) for the National Oceanic and Atmospheric Administration's (NOAA) national surface radiation budget network (SURFRAD) is summarized, and decadal results are presented. AOD is a measure of the extinction of the Sun's beam due to aerosols. Daily files of AOD for five spectral measurements in the visible and near-infrared have been produced for 1997-2006. Comparisons of SURFRAD daily AOD averages to NASA's Aerosol Robotic Network product at two of the stations were generally good. An AOD climatology for each SURFRAD station is presented as an annual time series of composite monthly means that represents a typical intra-annual AOD variation. Results are similar to previous U.S. climatologies in that the highest AOD magnitude and greatest variability occur in summer, the lowest AOD levels are in winter, and geographically, the highest-magnitude AOD is in the eastern United States. Springtime Asian dust intrusions show up as a secondary maximum at the western stations. A time series of nationwide annual means shows that 500-nm AOD has decreased over the United States by about 0.02 AOD units over the 10-year period. However, this decline is not statistically significant nor geographically consistent within the country. The eastern U.S. stations and westernmost station at Desert Rock, Nevada, show decreasing AOD, whereas the other two western stations show an increase that is attributed to an upsurge in wildfire activity in the last half of the decade.

  15. Aerosol climatology over the Mexico City basin: Characterization of optical properties

    NASA Astrophysics Data System (ADS)

    Carabali, Giovanni; Estévez, Héctor Raúl; Valdés-Barrón, Mauro; Bonifaz-Alfonzo, Roberto; Riveros-Rosas, David; Velasco-Herrera, Víctor Manuel; Vázquez-Gálvez, Felipe Adrián

    2017-09-01

    Climatology of Aerosol Optical Depth (AOD), Single Scattering Albedo (SSA), and aerosol particle-size distribution were analyzed using a 15-year (1999-2014) dataset from AErosol RObotic NETwork (AERONET) observations over the Mexico City (MC) basin. The atmosphere over this site is dominated by two main aerosol types, represented by urban/industrial pollution and biomass-burning particles. Due to the specific meteorological conditions within the basin, seasons are usually classified into three as follows: Dry Winter (DW) (November-February); Dry Spring (DS) (March-April), and the RAiny season (RA) (May-October), which are mentioned throughout this article. Using a CIMEL sun photometer, we conducted continuous observations over the MC urban area from January 1999 to December 2014. Aerosol Optical Depth (AOD), Ångström exponent (α440-870), Single Scattering Albedo (SSA), and aerosol particle-size distribution were derived from the observational data. The overall mean AOD500 during the 1999-2014 period was 0.34 ± 0.07. The monthly mean AOD reached a maximal value of 0.49 in May and a minimal value of 0.27 in February and March. The average α440-870 value for the period studied was 1.50 ± 0.16. The monthly average of α440-870 reached a minimal value of 1.32 in August and a maximal value of 1.61 in May. Average SSA at 440 nm was 0.89 throughout the observation period, indicating that aerosols over Mexico City are composed mainly of absorptive particles. Concentrations of fine- and coarse-mode aerosols over MC were highest in DS season compared with other seasons, especially for particles with radii measuring between 0.1 and 0.2 μm. Results from the Spectral De-convolution Algorithm (SDA) show that fine-mode aerosols dominated AOD variability in MC. In the final part of this article, we present a classification of aerosols in MC by using the graphical method proposed by Gobbi et al. (2007), which is based on the combined analysis of α and its spectral curvature

  16. Micropulse lidar-derived aerosol optical depth climatology at ARM sites worldwide

    NASA Astrophysics Data System (ADS)

    Kafle, D. N.; Coulter, R. L.

    2013-07-01

    This paper focuses on climatology of the vertical distribution of aerosol optical depth (AOD (z)) from micropulse lidar (MPL) observations for climatically different locations worldwide. For this, a large data set obtained by MPL systems operating at 532 nm during the 4 year period 2007-2010 was used to derive vertical profiles of AOD (z) by combining the corresponding AOD data as an input from an independent measurement using nearly colocated multifilter rotating shadowband radiometer (MFRSR) systems at five different U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Program sites—three permanent sites (SGP in north-central Oklahoma, at 36.6°N, 97.5°W, 320 m; TWP-Darwin in the tropical western Pacific, at 12.4°S, 130.9°E, 30 m; and NSA at Barrow on the North Slope of Alaska, at 71.3°N, 156.6°W, 8 m) and two mobile facility sites (GRW at Graciosa Island in the Azores, at 39°N, 28°W, 15 m; and FKB in the Black Forest of Germany, at 48.5°N, 8.4°E, 511 m). Therefore, amount of data used in this study is constrained by the availability of the MFRSR data. The MPL raw data were averaged for 30 s in time and 30 m in altitude. The diurnally averaged AOD (z) profiles from 4 years were combined to obtain a multiyear vertical profile of AOD (z) climatology at various ARM sites, including diurnal, day-to-day, and seasonal variabilities. Most aerosols were found to be confined to 0-2 km (approximately the planetary boundary layer region) at all sites; however, all sites exhibited measurable aerosols well above the mixed layer, with different height maxima. The entire data set demonstrates large day-to-day variability at all sites. However, there is no significant diurnal variation in AOD (z) at all sites. Significant interannual variability was observed at the SGP site. Clear seasonal variations in AOD (z) profiles exist for all five sites, but seasonal behavior was distinct. Moreover, the different seasonal variability for the lower level (0 to ~2

  17. A Climatologically Significant Aerosol Longwave Indirect Effect in the Arctic

    NASA Astrophysics Data System (ADS)

    Lubin, D.; Vogelmann, A.

    2006-12-01

    Analysis of Atmospheric Emitted Radiance Interferometer (AERI) data from the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Program North Slope of Alaska (NSA) site confirms a pervasive first indirect effect of aerosols in low-level stratiform clouds, which are the prevailing meteorological condition throughout the Arctic. The AERI longwave emission spectra under clouds of low to moderate optical depth (<8) are sensitive to both the effective droplet radius and the liquid water path, and can be used to retrieve both quantities. When supplemented by additional NSA sensor data, these AERI retrievals reveal a longwave surface flux enhancement of 8.2 Watts per square meter under liquid water clouds subject to aerosol entrainment versus similar clouds in clean air. Of this total enhancement revealed by co-located pyrgeometer data, 3.4 Watts per square meter can be readily attributed to the first indirect effect. This observed indirect effect occurs frequently during spring, but rarely during summer. The indirect effect's manifestation in the longwave is climatologically significant given that this part of the spectrum dominates the radiation budget at high latitudes throughout most of the year. Lubin, D., and A. M. Voglemann, Nature, 439, 453-456 (2006).

  18. A climatologically significant aerosol longwave indirect effect in the Arctic.

    PubMed

    Lubin, Dan; Vogelmann, Andrew M

    2006-01-26

    The warming of Arctic climate and decreases in sea ice thickness and extent observed over recent decades are believed to result from increased direct greenhouse gas forcing, changes in atmospheric dynamics having anthropogenic origin, and important positive reinforcements including ice-albedo and cloud-radiation feedbacks. The importance of cloud-radiation interactions is being investigated through advanced instrumentation deployed in the high Arctic since 1997 (refs 7, 8). These studies have established that clouds, via the dominance of longwave radiation, exert a net warming on the Arctic climate system throughout most of the year, except briefly during the summer. The Arctic region also experiences significant periodic influxes of anthropogenic aerosols, which originate from the industrial regions in lower latitudes. Here we use multisensor radiometric data to show that enhanced aerosol concentrations alter the microphysical properties of Arctic clouds, in a process known as the 'first indirect' effect. Under frequently occurring cloud types we find that this leads to an increase of an average 3.4 watts per square metre in the surface longwave fluxes. This is comparable to a warming effect from established greenhouse gases and implies that the observed longwave enhancement is climatologically significant.

  19. Three Dimensional Aerosol Climatology over India and the North Indian Ocean

    NASA Astrophysics Data System (ADS)

    Adams, A.; Zhang, C.

    2013-12-01

    Numerical models are indispensable tools to study aerosol effects on climate, including both aerosol direct and indirect radiative effects and their role in precipitation. But, agreement among the models has not been achieved, and thus it is not possible to accurately and confidently attain estimates of aerosol effects on climate. The lack of reliable knowledge on global three-dimensional (3D) aerosol climatology has prevented us from assessing the degree to which the disagreement in their aerosol climatic effects may come from differences of aerosol vertical structures in their simulations. To that end, we created a six year, global 3D extinction coefficient dataset for each aerosol species identifiable by the Level 2, Version 3, 5 km Aerosol Profile product from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) as a tool to improve 3D model representations. Here we describe the 3D structure of aerosol in the Middle East, India, and the Northern Indian Ocean and some of the interesting dynamical features responsible for the vertical structure and external mixing of aerosol species. One interesting feature in the 3D structure during boreal summer is a well-defined EC core located 0 - 10°N, 40°E - 90°E (Somalia across the Indian subcontinent), centered at 3 km. This is controlled by a shallow meridional circulation about the core. Additionally, the Somali Low-Level Jet exists at this location, but is usually located below the core (~850 mb). Another interesting feature is a strong EC core located 0 - 15°N, 60°E - 90°E below 0.5 km. Polluted dust (external mixture of dust and smoke) and marine aerosol are collocated in this area with maximum AODs of ~0.5 and ~0.2 respectively. Due to the wind stress over ocean, collocation of aerosol species, altitude, and lack of transport pathway for polluted dust, it is possible that this is an example of aerosol misclassification by

  20. Three-dimensional dust aerosol distribution and extinction climatology over northern Africa simulated with the ALADIN numerical prediction model from 2006 to 2010

    NASA Astrophysics Data System (ADS)

    Mokhtari, M.; Tulet, P.; Fischer, C.; Bouteloup, Y.; Bouyssel, F.; Brachemi, O.

    2015-08-01

    The seasonal cycle and optical properties of mineral dust aerosols in northern Africa were simulated for the period from 2006 to 2010 using the numerical atmospheric model ALADIN (Aire Limitée Adaptation dynamique Développement InterNational) coupled to the surface scheme SURFEX (SURFace EXternalisée). The particularity of the simulations is that the major physical processes responsible for dust emission and transport, as well as radiative effects, are taken into account on short timescales and at mesoscale resolution. The aim of these simulations is to quantify the dust emission and deposition, locate the major areas of dust emission and establish a climatology of aerosol optical properties in northern Africa. The mean monthly aerosol optical thickness (AOT) simulated by ALADIN is compared with the AOTs derived from the standard Dark Target (DT) and Deep Blue (DB) algorithms of the Aqua-MODIS (MODerate resolution Imaging Spectroradiometer) products over northern Africa and with a set of sun photometer measurements located at Banizoumbou, Cinzana, Soroa, Mbour and Cape Verde. The vertical distribution of dust aerosol represented by extinction profiles is also analysed using CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) observations. The annual dust emission simulated by ALADIN over northern Africa is 878 Tg year-1. The Bodélé Depression appears to be the main area of dust emission in northern Africa, with an average estimate of about 21.6 Tg year-1. The simulated AOTs are in good agreement with satellite and sun photometer observations. The positions of the maxima of the modelled AOTs over northern Africa match the observed positions, and the ALADIN simulations satisfactorily reproduce the various dust events over the 2006-2010 period. The AOT climatology proposed in this paper provides a solid database of optical properties and consolidates the existing climatology over this region derived from satellites, the AERONET network and regional climate

  1. A 10-year climatology of pollen aerosol for the continental United States: implications for aerosol-climate interactions

    NASA Astrophysics Data System (ADS)

    Wozniak, M. C.

    2016-12-01

    Our current understanding of biological particles and their role in the climate system is uncertain. Pollen, a primary biological aerosol particle, has been understudied in the context of climate and atmospheric science because of its coarse size (10-100 µm). Local coarse grain pollen concentrations can reach up to 10,000 grains m-3, and when ruptured by wet or turbulent atmospheric conditions, can produce fine particles (sub-pollen particles, 10-1000 nm) that may increase pollen's lifetime in the atmosphere. Therefore, pollen contributes to both coarse and fine particle loads in the atmosphere that may have climatic impacts. During peak pollen emissions season, what impacts does pollen have on aerosol concentrations in the atmosphere and their indirect forcing? Here we use a model of accurately timed and scaled pollen and sub-pollen particle emissions with climate-dependent phenological dates for four plant functional types (deciduous broadleaf, evergreen needleleaf, grass and ragweed) that dominate emissions across the continental United States. Terrestrial pollen emissions are coupled with the land component of a regional climate model (RegCM4-CLM), and are transported as atmospheric tracers that are allowed interact with radiation and clouds, accounting for the direct and indirect effects of pollen. A ten-year climatology of pollen emissions and climate interactions is calculated for both pollen grains and sub-pollen particles. Its implications for the local and overall radiation budget, aerosol-cloud-precipitation interactions and regional climate are discussed.

  2. Exploring Climatology and Long-Term Variations of Aerosols from NASA Reanalysis MERRA-2 with Giovanni

    NASA Technical Reports Server (NTRS)

    Shen, Suhung; Ostrenga, Dana; Vollmer, Bruce; Li, Zhanqing

    2016-01-01

    Dust plays important roles in energy cycle and climate variations. The dust deposition is the major source of iron in the open ocean, which is an essential micronutrient for phytoplankton growth and therefore may influence the ocean uptake of atmospheric CO2. Mineral dust can also act as fertilizer for forests over long time periods. Over 35 years of simulated global aerosol products from NASA atmospheric reanalysis, second Modern-Era Retrospective analysis for Research and Applications (MERRA-2) are available from NASA Goddard Earth Science Data and Information Services Center (GES DISC). The MERRA-2 covers the period 1980-present, continuing as an ongoing climate analysis. Aerosol assimilation is included throughout the period, using MODIS, MISR, AERONET, and AVHRR (in the pre-EOS period). The aerosols are assimilated by using MERRA-2 aerosol model, which interact directly with the radiation parameterization, and radiatively coupled with atmospheric model dynamics in the Goddard Earth Observing System Model, Version 5 (GEOS-5). Dust deposition data along with other major aerosol compositions (e.g. black carbon, sea salt, and sulfate, etc.) are simulated as dry and wet deposition, respectively. The hourly and monthly data are available at spatial resolution of 0.5ox0.625o (latitude x longitude). Quick data exploration of climatology and interannual variations of MERRA-2 aerosol can be done through the online visualization and analysis tool, Giovanni. This presentation, using dust deposition as an example, demonstrates a number of MERRA-2 data services at GES DISC. Global distributions of dust depositions, and their seasonal and inter-annual variations are investigated from MERRA-2 monthly aerosol products.

  3. Global volcanic aerosol properties derived from emissions, 1990-2014, using CESM1(WACCM): VOLCANIC AEROSOLS DERIVED FROM EMISSIONS

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Mills, Michael J.; Schmidt, Anja; Easter, Richard

    Accurate representation of global stratospheric aerosol properties from volcanic and non-volcanic sulfur emissions is key to understanding the cooling effects and ozone-loss enhancements of recent volcanic activity. Attribution of climate and ozone variability to volcanic activity is of particular interest in relation to the post-2000 slowing in the apparent rate of global average temperature increases, and variable recovery of the Antarctic ozone hole. We have developed a climatology of global aerosol properties from 1990 to 2014 calculated based on volcanic and non-volcanic emissions of sulfur sources. We have complied a database of volcanic SO2 emissions and plume altitudes for eruptionsmore » between 1990 and 2014, and a new prognostic capability for simulating stratospheric sulfate aerosols in version 5 of the Whole Atmosphere Community Climate Model, a component of the Community Earth System Model. Our climatology shows remarkable agreement with ground-based lidar observations of stratospheric aerosol optical depth (SAOD), and with in situ measurements of aerosol surface area density (SAD). These properties are key parameters in calculating the radiative and chemical effects of stratospheric aerosols. Our SAOD climatology represents a significant improvement over satellite-based analyses, which ignore aerosol extinction below 15 km, a region that can contain the vast majority of stratospheric aerosol extinction at mid- and high-latitudes. Our SAD climatology significantly improves on that provided for the Chemistry-Climate Model Initiative, which misses 60% of the SAD measured in situ. Our climatology of aerosol properties is publicly available on the Earth System Grid.« less

  4. A climatology of fine absorbing biomass burning, urban and industrial aerosols detected from satellites

    NASA Astrophysics Data System (ADS)

    Kalaitzi, Nikoleta; Hatzianastassiou, Nikos; Gkikas, Antonis; Papadimas, Christos D.; Torres, Omar; Mihalopoulos, Nikos

    2017-04-01

    Natural biomass burning (BB) along with anthropogenic urban and industrial aerosol particles, altogether labeled here as BU aerosols, contain black and brown carbon which both absorb strongly the solar radiation. Thus, BU aerosols warm significantly the atmosphere also causing adjustments to cloud properties, which traditionally are known as cloud indirect and semi-direct effects. Given the role of the effects of BU aerosols for contemporary and future climate change, and the uncertainty associated with BU, both ascertained by the latest IPCC reports, there is an urgent need for improving our knowledge on the spatial and temporal variability of BU aerosols all over the globe. Over the last few decades, thanks to the rapid development of satellite observational techniques and retrieval algorithms it is now possible to detect BU aerosols based on satellite measurements. However, care must be taken in order to ensure the ability to distinguish BU from other aerosol types usually co-existing in the Earth's atmosphere. In the present study, an algorithm is presented, based on a synergy of different satellite measurements, aiming to identify and quantify BU aerosols over the entire globe and during multiple years. The objective is to build a satellite-based climatology of BU aerosols intended for use for various purposes. The produced regime, namely the spatial and temporal variability of BU aerosols, emphasizes the BU frequency of occurrence and their intensity, in terms of aerosol optical depth (AOD). The algorithm is using the following aerosol optical properties describing the size and atmospheric loading of BU aerosols: (i) spectral AOD, (ii) Ångström Exponent (AE), (iii) Fine Fraction (FF) and (iv) Aerosol Index (AI). The relevant data are taken from Collection 006 MODIS-Aqua, except for AI which is taken from OMI-Aura. The identification of BU aerosols by the algorithm is based on a specific thresholding technique, with AI≥1.5, AE≥1.2 and FF≥0.6 threshold

  5. Comparison of MADE3-simulated and observed aerosol distributions with a focus on aerosol vertical profiles

    NASA Astrophysics Data System (ADS)

    Kaiser, Christopher; Hendricks, Johannes; Righi, Mattia; Jöckel, Patrick

    2016-04-01

    The reliability of aerosol radiative forcing estimates from climate models depends on the accuracy of simulated global aerosol distribution and composition, as well as on the models' representation of the aerosol-cloud and aerosol-radiation interactions. To help improve on previous modeling studies, we recently developed the new aerosol microphysics submodel MADE3 that explicitly tracks particle mixing state in the Aitken, accumulation, and coarse mode size ranges. We implemented MADE3 into the global atmospheric chemistry general circulation model EMAC and evaluated it by comparison of simulated aerosol properties to observations. Compared properties include continental near-surface aerosol component concentrations and size distributions, continental and marine aerosol vertical profiles, and nearly global aerosol optical depth. Recent studies have shown the specific importance of aerosol vertical profiles for determination of the aerosol radiative forcing. Therefore, our focus here is on the evaluation of simulated vertical profiles. The observational data is taken from campaigns between 1990 and 2011 over the Pacific Ocean, over North and South America, and over Europe. The datasets include black carbon and total aerosol mass mixing ratios, as well as aerosol particle number concentrations. Compared to other models, EMAC with MADE3 yields good agreement with the observations - despite a general high bias of the simulated mass mixing ratio profiles. However, BC concentrations are generally overestimated by many models in the upper troposphere. With MADE3 in EMAC, we find better agreement of the simulated BC profiles with HIPPO data than the multi-model average of the models that took part in the AeroCom project. There is an interesting difference between the profiles from individual campaigns and more "climatological" datasets. For instance, compared to spatially and temporally localized campaigns, the model simulates a more continuous decline in both total

  6. The Global Precipitation Climatology Project (GPCP) Combined Precipitation Dataset

    NASA Technical Reports Server (NTRS)

    Huffman, George J.; Adler, Robert F.; Arkin, Philip; Chang, Alfred; Ferraro, Ralph; Gruber, Arnold; Janowiak, John; McNab, Alan; Rudolf, Bruno; Schneider, Udo

    1997-01-01

    The Global Precipitation Climatology Project (GPCP) has released the GPCP Version 1 Combined Precipitation Data Set, a global, monthly precipitation dataset covering the period July 1987 through December 1995. The primary product in the dataset is a merged analysis incorporating precipitation estimates from low-orbit-satellite microwave data, geosynchronous-orbit -satellite infrared data, and rain gauge observations. The dataset also contains the individual input fields, a combination of the microwave and infrared satellite estimates, and error estimates for each field. The data are provided on 2.5 deg x 2.5 deg latitude-longitude global grids. Preliminary analyses show general agreement with prior studies of global precipitation and extends prior studies of El Nino-Southern Oscillation precipitation patterns. At the regional scale there are systematic differences with standard climatologies.

  7. General Climatology 3

    NASA Astrophysics Data System (ADS)

    Hartmann, Dennis L.

    General Climatology 3 is volume 3 of the series World Survey of Climatology, which consists of 15 volumes containing review articles on a broad range of topics. General Climatology 3 contains four chapters: ‘Human Bioclimatology,’ ‘Agricultural Climatology,’ ‘City Climate,’ and ‘Technical Climatology.’ Each of these chapters will be briefly described here.‘Human Bioclimatology,’ the first chapter, was authored by E. Flach and provides a survey of the effects on the human organism of the physical conditions at the earth's surface. It contains four main sections. A section entitled ‘Light and Life’ deals with the effects of solar radiation on man and contains much interesting information on the response of the human eye and human skin to radiation at various frequencies. ‘Air and Life’ discusses the composition of air and its effect on human health and performance, including discussions of the effects of altitude, aerosols, and noxious trace gases. ‘Temperature and Life’ discusses how the body responds to temperature and how it maintains its heat budget under the variety of conditions to which it falls subject and considerable discussion is given to objective ways to characterize air conditions that give an accurate measure of their impact on the body. This discussion leads naturally into the final section, ‘Bioclimatological Evaluation Systems,’ which addresses the problem of how to classify a particular site according to its overall suitability to human habitation.

  8. aerosol radiative effects and forcing: spatial and temporal distributions

    NASA Astrophysics Data System (ADS)

    Kinne, Stefan

    2014-05-01

    A monthly climatology for aerosol optical properties based on a synthesis from global modeling and observational data has been applied to illustrate spatial distributions and global averages of aerosol radiative impacts. With the help of a pre-industrial reference for aerosol optical properties from global modeling, also the aerosol direct forcing (ca -0.35W/m2 globally and annual averaged) and their spatial and seasonal distributions and contributions by individual aerosol components are estimated. Finally, CCN and IN concentrations associated with this climatology are applied to estimate aerosol indirect effects and forcing.

  9. Atmosphere aerosol satellite project Aerosol-UA

    NASA Astrophysics Data System (ADS)

    Milinevsky, Gennadi; Yatskiv, Yaroslav; Syniavskyi, Ivan; Bovchaliuk, Andrii; Degtyaryov, Oleksandr; Sosonkin, Mikhail; Mishchenko, Michael; Danylevsky, Vassyl; Ivanov, Yury; Oberemok, Yevgeny; Masley, Volodymyr; Rosenbush, Vera; Moskalev, Sergii

    2017-04-01

    channels of the MSIP are the intensity channels that serve to obtain images in eight spectral wavebands to retrieve the aerosol optical depth. The main feature of the each MSIP channel is the splitting of the image by a special prism-splitter to four images on the same CCD detector. In that way we can simultaneously measure four polarization components at 0°, 45°, 90° and 135° as images in each of three polarization channels. One of the special features of ScanPol/MSIP concept is calibration of the MSIP using ScanPol data in the same field-of-view with 1% expected polarization accuracy. The Aerosol-UA experiment is planned to be launched in 2020 at the new satellite platform YuzhSat developed in the Yuzhnoye Design Office. The GRASP algorithm (Dubovik et al. 2014, doi: 10.1117/2.1201408.005558) is planned for Aerosol-UA data processing and AERONET sun photometers observations for validation. Acknowledgements. The work was partly supported by the Special Complex Program for Space Research 2012-2016 of the National Academy of Sciences of Ukraine, by the project 16BF051-02 of the Taras Shevchenko National University of Kyiv, and by the grant of the State Fund for Fundamental Research, project F73/115-2016.

  10. Estimating Climatological Bias Errors for the Global Precipitation Climatology Project (GPCP)

    NASA Technical Reports Server (NTRS)

    Adler, Robert; Gu, Guojun; Huffman, George

    2012-01-01

    A procedure is described to estimate bias errors for mean precipitation by using multiple estimates from different algorithms, satellite sources, and merged products. The Global Precipitation Climatology Project (GPCP) monthly product is used as a base precipitation estimate, with other input products included when they are within +/- 50% of the GPCP estimates on a zonal-mean basis (ocean and land separately). The standard deviation s of the included products is then taken to be the estimated systematic, or bias, error. The results allow one to examine monthly climatologies and the annual climatology, producing maps of estimated bias errors, zonal-mean errors, and estimated errors over large areas such as ocean and land for both the tropics and the globe. For ocean areas, where there is the largest question as to absolute magnitude of precipitation, the analysis shows spatial variations in the estimated bias errors, indicating areas where one should have more or less confidence in the mean precipitation estimates. In the tropics, relative bias error estimates (s/m, where m is the mean precipitation) over the eastern Pacific Ocean are as large as 20%, as compared with 10%-15% in the western Pacific part of the ITCZ. An examination of latitudinal differences over ocean clearly shows an increase in estimated bias error at higher latitudes, reaching up to 50%. Over land, the error estimates also locate regions of potential problems in the tropics and larger cold-season errors at high latitudes that are due to snow. An empirical technique to area average the gridded errors (s) is described that allows one to make error estimates for arbitrary areas and for the tropics and the globe (land and ocean separately, and combined). Over the tropics this calculation leads to a relative error estimate for tropical land and ocean combined of 7%, which is considered to be an upper bound because of the lack of sign-of-the-error canceling when integrating over different areas with a

  11. Recent Trends of the Tropical Hydrological Cycle Inferred from Global Precipitation Climatology Project and International Satellite Cloud Climatology Project data

    NASA Technical Reports Server (NTRS)

    Zhou, Y. P.; Xu, Kuan-Man; Sud, Y. C.; Betts, A. K.

    2011-01-01

    Scores of modeling studies have shown that increasing greenhouse gases in the atmosphere impact the global hydrologic cycle; however, disagreements on regional scales are large, and thus the simulated trends of such impacts, even for regions as large as the tropics, remain uncertain. The present investigation attempts to examine such trends in the observations using satellite data products comprising Global Precipitation Climatology Project precipitation and International Satellite Cloud Climatology Project cloud and radiation. Specifically, evolving trends of the tropical hydrological cycle over the last 20-30 years were identified and analyzed. The results show (1) intensification of tropical precipitation in the rising regions of the Walker and Hadley circulations and weakening over the sinking regions of the associated overturning circulation; (2) poleward shift of the subtropical dry zones (up to 2deg/decade in June-July-August (JJA) in the Northern Hemisphere and 0.3-0.7deg/decade in June-July-August and September-October-November in the Southern Hemisphere) consistent with an overall broadening of the Hadley circulation; and (3) significant poleward migration (0.9-1.7deg/decade) of cloud boundaries of Hadley cell and plausible narrowing of the high cloudiness in the Intertropical Convergence Zone region in some seasons. These results support findings of some of the previous studies that showed strengthening of the tropical hydrological cycle and expansion of the Hadley cell that are potentially related to the recent global warming trends.

  12. The "Deep Blue" Aerosol Project at NASA GSFC

    NASA Technical Reports Server (NTRS)

    Sayer, Andrew; Hsu, N. C.; Lee, J.; Bettenhausen, C.; Carletta, N.; Chen, S.; Esmaili, R.

    2016-01-01

    Atmospheric aerosols such as mineral dust, wildfire smoke, sea spray, and volcanic ash are of interest for a variety of reasons including public health, climate change, hazard avoidance, and more. Deep Blue is a project which uses satellite observations of the Earth from sensors such as SeaWiFS, MODIS, and VIIRS to monitor the global aerosol burden. This talk will cover some basics about aerosols and the principles of aerosol remote sensing, as well as discussing specific results and future directions for the Deep Blue project.

  13. A 4-D Climatology (1979-2009) of the Monthly Tropospheric Aerosol Optical Depth Distribution over the Mediterranean Region from a Comparative Evaluation and Blending of Remote Sensing and Model Products

    NASA Technical Reports Server (NTRS)

    Nabat, P.; Somot, S.; Mallet, M.; Chiapello, I; Morcrette, J. J.; Solomon, F.; Szopa, S.; Dulac, F; Collins, W.; Ghan, S.; hide

    2013-01-01

    Since the 1980s several spaceborne sensors have been used to retrieve the aerosol optical depth (AOD) over the Mediterranean region. In parallel, AOD climatologies coming from different numerical model simulations are now also available, permitting to distinguish the contribution of several aerosol types to the total AOD. In this work, we perform a comparative analysis of this unique multiyear database in terms of total AOD and of its apportionment by the five main aerosol types (soil dust, seasalt, sulfate, black and organic carbon). We use 9 different satellite-derived monthly AOD products: NOAA/AVHRR, SeaWiFS (2 products), TERRA/MISR, TERRA/MODIS, AQUA/MODIS, ENVISAT/MERIS, PARASOL/POLDER and MSG/SEVIRI, as well as 3 more historical datasets: NIMBUS7/CZCS, TOMS (onboard NIMBUS7 and Earth- Probe) and METEOSAT/MVIRI. Monthly model datasets include the aerosol climatology from Tegen et al. (1997), the climate-chemistry models LMDz-OR-INCA and RegCM-4, the multi-model mean coming from the ACCMIP exercise, and the reanalyses GEMS and MACC. Ground-based Level- 2 AERONET AOD observations from 47 stations around the basin are used here to evaluate the model and satellite data. The sensor MODIS (on AQUA and TERRA) has the best average AOD scores over this region, showing a relevant spatio-temporal variability and highlighting high dust loads over Northern Africa and the sea (spring and summer), and sulfate aerosols over continental Europe (summer). The comparison also shows limitations of certain datasets (especially MERIS and SeaWiFS standard products). Models reproduce the main patterns of the AOD variability over the basin. The MACC reanalysis is the closest to AERONET data, but appears to underestimate dust over Northern Africa, where RegCM-4 is found closer to MODIS thanks to its interactive scheme for dust emissions. The vertical dimension is also investigated using the CALIOP instrument. This study confirms differences of vertical distribution between dust

  14. New Satellite Project Aerosol-UA: Remote Sensing of Aerosols in the Terrestrial Atmosphere

    NASA Technical Reports Server (NTRS)

    Milinevsky, G.; Yatskiv, Ya.; Degtyaryov, O.; Syniavskyi, I.; Mishchenko, Michael I.; Rosenbush, V.; Ivanov, Yu.; Makarov, A.; Bovchaliuk, A.; Danylevsky, V.; hide

    2016-01-01

    We discuss the development of the Ukrainian space project Aerosol-UA which has the following three main objectives: (1) to monitor the spatial distribution of key characteristics of terrestrial tropospheric and stratospheric aerosols; (2) to provide a comprehensive observational database enabling accurate quantitative estimates of the aerosol contribution to the energy budget of the climate system; and (3) quantify the contribution of anthropogenic aerosols to climate and ecological processes. The remote sensing concept of the project is based on precise orbital measurements of the intensity and polarization of sunlight scattered by the atmosphere and the surface with a scanning polarimeter accompanied by a wide-angle multispectral imager-polarimeter. Preparations have already been made for the development of the instrument suite for the Aerosol-UA project, in particular, of the multi-channel scanning polarimeter (ScanPol) designed for remote sensing studies of the global distribution of aerosol and cloud properties (such as particle size, morphology, and composition) in the terrestrial atmosphere by polarimetric and spectrophotometric measurements of the scattered sunlight in a wide range of wavelengths and viewing directions from which a scene location is observed. ScanPol is accompanied by multispectral wide-angle imager-polarimeter (MSIP) that serves to collect information on cloud conditions and Earths surface image. Various components of the polarimeter ScanPol have been prototyped, including the opto-mechanical and electronic assemblies and the scanning mirror controller. Preliminary synthetic data simulations for the retrieval of aerosol parameters over land surfaces have been performed using the Generalized Retrieval of Aerosol and Surface Properties (GRASP) algorithm. Methods for the validation of satellite data using ground-based observations of aerosol properties are also discussed. We assume that designing, building, and launching into orbit a multi

  15. A generalized formulation for downscaling data based on Fourier Transform and inversion: Mathematical rationale and application to the Max-Planck-Institute aerosol climatology data

    NASA Astrophysics Data System (ADS)

    Zhang, Taiping; Stackhouse, Paul W.; Gupta, Shashi K.; Cox, Stephen J.; Mikovitz, J. Colleen

    2017-02-01

    Occasionally, a need arises to downscale a time series of data from a coarse temporal resolution to a finer one, a typical example being from monthly means to daily means. For this case, daily means derived as such are used as inputs of climatic or atmospheric models so that the model results may exhibit variance on the daily time scale and retain the monthly mean of the original data set without an abrupt change from the end of one month to the beginning of the next. Different methods have been developed which often need assumptions, free parameters and the solution of simultaneous equations. Here we derive a generalized formulation by means of Fourier transform and inversion so that it can be used to directly compute daily means from a series of an arbitrary number of monthly means. The formulation can be used to transform any coarse temporal resolution to a finer one. From the derived results, the original data can be recovered almost identically. As a real application, we use this method to derive the daily counterpart of the MAC-v1 aerosol climatology that provides monthly mean aerosol properties for 18 shortwave bands and 12 longwave bands for the years from 1860 to 2100. The derived daily means are to be used as inputs of the shortwave and longwave algorithms of the NASA GEWEX SRB project.

  16. Indirect aerosol effect increases CMIP5 models projected Arctic warming

    DOE PAGES

    Chylek, Petr; Vogelsang, Timothy J.; Klett, James D.; ...

    2016-02-20

    Phase 5 of the Coupled Model Intercomparison Project (CMIP5) climate models’ projections of the 2014–2100 Arctic warming under radiative forcing from representative concentration pathway 4.5 (RCP4.5) vary from 0.9° to 6.7°C. Climate models with or without a full indirect aerosol effect are both equally successful in reproducing the observed (1900–2014) Arctic warming and its trends. However, the 2014–2100 Arctic warming and the warming trends projected by models that include a full indirect aerosol effect (denoted here as AA models) are significantly higher (mean projected Arctic warming is about 1.5°C higher) than those projected by models without a full indirect aerosolmore » effect (denoted here as NAA models). The suggestion is that, within models including full indirect aerosol effects, those projecting stronger future changes are not necessarily distinguishable historically because any stronger past warming may have been partially offset by stronger historical aerosol cooling. In conclusion, the CMIP5 models that include a full indirect aerosol effect follow an inverse radiative forcing to equilibrium climate sensitivity relationship, while models without it do not.« less

  17. Indirect aerosol effect increases CMIP5 models projected Arctic warming

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Chylek, Petr; Vogelsang, Timothy J.; Klett, James D.

    Phase 5 of the Coupled Model Intercomparison Project (CMIP5) climate models’ projections of the 2014–2100 Arctic warming under radiative forcing from representative concentration pathway 4.5 (RCP4.5) vary from 0.9° to 6.7°C. Climate models with or without a full indirect aerosol effect are both equally successful in reproducing the observed (1900–2014) Arctic warming and its trends. However, the 2014–2100 Arctic warming and the warming trends projected by models that include a full indirect aerosol effect (denoted here as AA models) are significantly higher (mean projected Arctic warming is about 1.5°C higher) than those projected by models without a full indirect aerosolmore » effect (denoted here as NAA models). The suggestion is that, within models including full indirect aerosol effects, those projecting stronger future changes are not necessarily distinguishable historically because any stronger past warming may have been partially offset by stronger historical aerosol cooling. In conclusion, the CMIP5 models that include a full indirect aerosol effect follow an inverse radiative forcing to equilibrium climate sensitivity relationship, while models without it do not.« less

  18. A 4-D Climatology (1979-2009) of the Monthly Tropospheric Aerosol Optical Depth Distribution over the Mediterranean Region from a Comparative Evaluation and Blending of Remote Sensing and Model Products

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nabat, P.; Somot, S.; Mallet, M.

    Since the 1980s several spaceborne sensors have been used to retrieve the aerosol optical depth (AOD) over the Mediterranean region. In parallel, AOD climatologies coming from different numerical model simulations are now also available, permitting to distinguish the contribution of several aerosol types to the total AOD. In this work, we perform a comparative analysis of this unique multiyear database in terms of total AOD and of its apportionment by the five main aerosol types (soil dust, seasalt, sulfate, black and organic carbon). We use 9 different satellite-derived monthly AOD products: NOAA/AVHRR, SeaWiFS (2 products), TERRA/MISR, TERRA/MODIS, AQUA/MODIS, ENVISAT/MERIS, PARASOL/POLDERmore » and MSG/SEVIRI, as well as 3 more historical datasets: NIMBUS7/CZCS, TOMS (onboard NIMBUS7 and Earth- Probe) and METEOSAT/MVIRI. Monthly model datasets include the aerosol climatology from Tegen et al. (1997), the climate-chemistry models LMDz-OR-INCA and RegCM-4, the multi-model mean coming from the ACCMIP exercise, and the reanalyses GEMS and MACC. Ground-based Level- 2 AERONET AOD observations from 47 stations around the basin are used here to evaluate the model and satellite data. The sensor MODIS (on AQUA and TERRA) has the best average AOD scores over this region, showing a relevant spatiotemporal variability and highlighting high dust loads over Northern Africa and the sea (spring and summer), and sulfate aerosols over continental Europe (summer). The comparison also shows limitations of certain datasets (especially MERIS and SeaWiFS standard products). Models reproduce the main patterns of the AOD variability over the basin. The MACC reanalysis is the closest to AERONET data, but appears to underestimate dust over Northern Africa, where RegCM-4 is found closer to MODIS thanks to its interactive scheme for dust emissions. The vertical dimension is also investigated using the CALIOP instrument. This study confirms differences of vertical distribution between dust

  19. simplified aerosol representations in global modeling

    NASA Astrophysics Data System (ADS)

    Kinne, Stefan; Peters, Karsten; Stevens, Bjorn; Rast, Sebastian; Schutgens, Nick; Stier, Philip

    2015-04-01

    The detailed treatment of aerosol in global modeling is complex and time-consuming. Thus simplified approaches are investigated, which prescribe 4D (space and time) distributions of aerosol optical properties and of aerosol microphysical properties. Aerosol optical properties are required to assess aerosol direct radiative effects and aerosol microphysical properties (in terms of their ability as aerosol nuclei to modify cloud droplet concentrations) are needed to address the indirect aerosol impact on cloud properties. Following the simplifying concept of the monthly gridded (1x1 lat/lon) aerosol climatology (MAC), new approaches are presented and evaluated against more detailed methods, including comparisons to detailed simulations with complex aerosol component modules.

  20. What is the "Clim-Likely" aerosol product?

    Atmospheric Science Data Center

    2014-12-08

    ... identifying a range of components and mixtures for the MISR Standard Aerosol Retrieval Algorithm climatology, and as one standard against ... retrieval results. Six component aerosols included in the model were medium and coarse mode mineral dust, sulfate, sea salt, black ...

  1. Evaluation and Applications of Cloud Climatologies from CALIOP

    NASA Technical Reports Server (NTRS)

    Winker, David; Getzewitch, Brian; Vaughan, Mark

    2008-01-01

    Clouds have a major impact on the Earth radiation budget and differences in the representation of clouds in global climate models are responsible for much of the spread in predicted climate sensitivity. Existing cloud climatologies, against which these models can be tested, have many limitations. The CALIOP lidar, carried on the CALIPSO satellite, has now acquired over two years of nearly continuous cloud and aerosol observations. This dataset provides an improved basis for the characterization of 3-D global cloudiness. Global average cloud cover measured by CALIOP is about 75%, significantly higher than for existing cloud climatologies due to the sensitivity of CALIOP to optically thin cloud. Day/night biases in cloud detection appear to be small. This presentation will discuss detection sensitivity and other issues associated with producing a cloud climatology, characteristics of cloud cover statistics derived from CALIOP data, and applications of those statistics.

  2. Synergetic use of Aerosol Robotic Network (AERONET) and Moderate Image Spectrometer (MODIS)

    NASA Technical Reports Server (NTRS)

    Kaufman, Y.

    2004-01-01

    I shall describe several distinct modes in which AERONET data are used in conjunction with MODIS data to evaluate the global aerosol system and its impact on climate. These includes: 1) Evaluation of the aerosol diurnal cycle not available from MODIS, and the relationship between the aerosol properties derived from MODIS and the daily average of these properties; 2) Climatology of the aerosol size distribution and single scattering albedo. The climatology is used to formulate the assumptions used in the MODIS look up tables used in the inversion of MODIS data; 3) Measurement of the aerosol effect on irradiation of the surface, this is used in conjunction with the MODIS evaluation of the aerosol effect at the TOA; and 4) Assessment of the aerosol baseline on top off which the satellite data are used to find the amount of dust or anthropogenic aerosol.

  3. Trends in aerosol optical depth in the Russian Arctic and their links with synoptic climatology.

    PubMed

    Shahgedanova, Maria; Lamakin, Mikhail

    2005-04-01

    Temporal and spatial variability of aerosol optical depth (AOD) are examined using observations of direct solar radiation in the Eurasian Arctic for 1940-1990. AOD is estimated using empirical methods for 14 stations located between 66.2 degrees N and 80.6 degrees N, from the Kara Sea to the Chukchi Sea. While AOD exhibits a well-known springtime maximum and summertime minimum at all stations, atmospheric turbidity is higher in spring in the western (Kara-Laptev) part of the Eurasian Arctic. Between June and August, the eastern (East Siberian-Chukchi) sector experiences higher transparency than the western part. A statistically significant positive trend in AOD was observed in the Kara-Laptev sector between the late 1950s and the early 1980s predominantly in spring when pollution-derived aerosol dominates the Arctic atmosphere but not in the eastern sector. Although all stations are remote, those with positive trends are located closer to the anthropogenic sources of air pollution. By contrast, a widespread decline in AOD was observed between 1982 and 1990 in the eastern Arctic in spring but was limited to two sites in the western Arctic. These results suggest that the post-1982 decline in anthropogenic emissions in Europe and the former Soviet Union has had a limited effect on aerosol load in the Arctic. The post-1982 negative trends in AOD in summer, when marine aerosol is present in the atmosphere, were more common in the west. The relationships between AOD and atmospheric circulation are examined using a synoptic climatology approach. In spring, AOD depends primarily on the strength and direction of air flow. Thus strong westerly and northerly flows result in low AOD values in the East Siberian-Chukchi sector. By contrast, strong southerly flow associated with the passage of depressions results in high AOD in the Kara-Laptev sector and trajectory analysis points to the contribution of industrial regions of the sub-Arctic. In summer, low pressure gradient or

  4. Modelling the background aerosol climatologies (1989-2010) for the Mediterranean basin

    NASA Astrophysics Data System (ADS)

    Jimenez-Guerrero, Pedro; Jerez, Sonia

    2014-05-01

    seasonally; here the sea spray clearly follows the wind speed variation. The results confirm the capability of the modelling strategies to reproduce the particulate matter levels, composition and variation in the Mediterranean area. This kind of information is useful for establishing improvement strategies for the prediction aerosols and to achieve the standards set in European Directives for modeling applications. Kulmala, M., Asmi, A., Lappalainen, H.K., Carslaw, K.S., Pöschl, U., Baltensperger, U. Hov, O., Brenquier, J.-L., Pandis, S.N., Facchini, M.C., Hanson, H.-C., Wiedensohler, A., O'Dowd, C.D., 2009. Introduction: European Integrated Project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI) - integrating aerosol research from nano to global scales. Amos. Chem. Phys., 9, 2825-2841. Querol, X., Alastuey, A., Pey, J., Cusack, M., Pérez, N., Mihalopoulos, N., Theodosi, C., Gerasopoulos, E., Kubilay, N., Koçak, M., 2009. Variability in regional background aerosols within the Mediterranean. Atmos. Chem. Phys., 9, 4575-4591.

  5. Impacts of increasing the aerosol complexity in the Met Office global NWP model

    NASA Astrophysics Data System (ADS)

    Mulcahy, J. P.; Walters, D. N.; Bellouin, N.; Milton, S. F.

    2013-11-01

    Inclusion of the direct and indirect radiative effects of aerosols in high resolution global numerical weather prediction (NWP) models is being increasingly recognised as important for the improved accuracy of short-range weather forecasts. In this study the impacts of increasing the aerosol complexity in the global NWP configuration of the Met Office Unified Model (MetUM) are investigated. A hierarchy of aerosol representations are evaluated including three dimensional monthly mean speciated aerosol climatologies, fully prognostic aerosols modelled using the CLASSIC aerosol scheme and finally, initialised aerosols using assimilated aerosol fields from the GEMS project. The prognostic aerosol schemes are better able to predict the temporal and spatial variation of atmospheric aerosol optical depth, which is particularly important in cases of large sporadic aerosol events such as large dust storms or forest fires. Including the direct effect of aerosols improves model biases in outgoing longwave radiation over West Africa due to a better representation of dust. However, uncertainties in dust optical properties propogate to its direct effect and the subsequent model response. Inclusion of the indirect aerosol effects improves surface radiation biases at the North Slope of Alaska ARM site due to lower cloud amounts in high latitude clean air regions. This leads to improved temperature and height forecasts in this region. Impacts on the global mean model precipitation and large-scale circulation fields were found to be generally small in the short range forecasts. However, the indirect aerosol effect leads to a strengthening of the low level monsoon flow over the Arabian Sea and Bay of Bengal and an increase in precipitation over Southeast Asia. Regional impacts on the African Easterly Jet (AEJ) are also presented with the large dust loading in the aerosol climatology enhancing of the heat low over West Africa and weakening the AEJ. This study highlights the importance

  6. Sensitivity of aerosol radiative forcing efficiency to the coarse mode contributions across aerosol regimes

    NASA Astrophysics Data System (ADS)

    McComiskey, A. C.; Telg, H.; Sheridan, P. J.; Kassianov, E.

    2017-12-01

    The coarse mode contribution to the aerosol radiative effect in a range of clean and turbid aerosol regimes has not been well quantified. While the coarse-mode radiative effect in turbid conditions is generally assumed to be consequential, the effect in clean conditions has likely been underestimated. We survey ground-based in situ measurements of the coarse mode fraction of aerosol optical properties measured around the globe over the past 20 years by the DOE Atmospheric Radiation Measurement Facility and the NOAA Global Monitoring Division. The aerosol forcing efficiency is presented, allowing an evaluation of where the aerosol coarse mode might be climatologically significant.

  7. Challenges to producing a long-term stratospheric aerosol climatology for chemistry and climate

    NASA Astrophysics Data System (ADS)

    Thomason, Larry; Vernier, Jean-Paul; Bourassa, Adam; Rieger, Landon; Luo, Beiping; Peter, Thomas; Arfeuille, Florian

    2016-04-01

    Stratospheric aerosol data sets are key inputs for climate models (GCMs, CCMs) particularly for understanding the role of volcanoes on climate and as a surrogate for understanding the potential of human-derived stratospheric aerosol as mitigation for global warming. In addition to supporting activities of individual climate models, the data sets also act as a historical input to the activities of SPARC's Chemistry-Climate Model Initiative (CCMI) and the World Climate Research Programme's Coupled Model Intercomparison Project (CMIP). One such data set was produced in 2004 as a part of the SPARC Assessment of Stratospheric Aerosol Properties (ASAP), extending from 1979 and 2004. It was primarily constructed from the Stratospheric Aerosol and Gas Experiment series of instruments but supplemented by data from other space-based sources and a number of ground-based and airborne instruments. Updates to this data set have expanded the timeframe to span from 1850 through 2014 through the inclusion of data from additional sources, such as photometer data and ice core analyses. Fundamentally, there are limitations to the reliability of the optical properties of aerosol inferred from even the most complete single instrument data sets. At the same time, the heterogeneous nature of the underlying data to this historical data set produces considerable challenges to the production of a climate data set which is both homogeneous and reliable throughout its timespan. In this presentation, we will discuss the impact of this heterogeneity showing specific examples such as the SAGE II to OSIRIS/CALIPSO transition in 2005. Potential solutions to these issues will also be discussed.

  8. The Global Precipitation Climatology Project: First Algorithm Intercomparison Project

    NASA Technical Reports Server (NTRS)

    Arkin, Phillip A.; Xie, Pingping

    1994-01-01

    The Global Precipitation Climatology Project (GPCP) was established by the World Climate Research Program to produce global analyses of the area- and time-averaged precipitation for use in climate research. To achieve the required spatial coverage, the GPCP uses simple rainfall estimates derived from IR and microwave satellite observations. In this paper, we describe the GPCP and its first Algorithm Intercomparison Project (AIP/1), which compared a variety of rainfall estimates derived from Geostationary Meteorological Satellite visible and IR observations and Special Sensor Microwave/Imager (SSM/I) microwave observations with rainfall derived from a combination of radar and raingage data over the Japanese islands and the adjacent ocean regions during the June and mid-July through mid-August periods of 1989. To investigate potential improvements in the use of satellite IR data for the estimation of large-scale rainfall for the GPCP, the relationship between rainfall and the fractional coverage of cold clouds in the AIP/1 dataset is examined. Linear regressions between fractional coverage and rainfall are analyzed for a number of latitude-longitude areas and for a range of averaging times. The results show distinct differences in the character of the relationship for different portions of the area. These results suggest that the simple IR-based estimation technique currently used in the GPCP can be used to estimate rainfall for global tropical and subtropical areas, provided that a method for adjusting the proportional coefficient for varying areas and seasons can be determined.

  9. An aerosol climatology for a rapidly growing arid region (southern Arizona): Major aerosol species and remotely sensed aerosol properties

    NASA Astrophysics Data System (ADS)

    Sorooshian, Armin; Wonaschütz, Anna; Jarjour, Elias G.; Hashimoto, Bryce I.; Schichtel, Bret A.; Betterton, Eric A.

    2011-10-01

    This study reports a comprehensive characterization of atmospheric aerosol particle properties in relation to meteorological and back trajectory data in the southern Arizona region, which includes two of the fastest growing metropolitan areas in the United States (Phoenix and Tucson). Multiple data sets (MODIS, AERONET, OMI/TOMS, MISR, GOCART, ground-based aerosol measurements) are used to examine monthly trends in aerosol composition, aerosol optical depth (AOD), and aerosol size. Fine soil, sulfate, and organics dominate PM2.5 mass in the region. Dust strongly influences the region between March and July owing to the dry and hot meteorological conditions and back trajectory patterns. Because monsoon precipitation begins typically in July, dust levels decrease, while AOD, sulfate, and organic aerosol reach their maximum levels because of summertime photochemistry and monsoon moisture. Evidence points to biogenic volatile organic compounds being a significant source of secondary organic aerosol in this region. Biomass burning also is shown to be a major contributor to the carbonaceous aerosol budget in the region, leading to enhanced organic and elemental carbon levels aloft at a sky-island site north of Tucson (Mt. Lemmon). Phoenix exhibits different monthly trends for aerosol components in comparison with the other sites owing to the strong influence of fossil carbon and anthropogenic dust. Trend analyses between 1988 and 2009 indicate that the strongest statistically significant trends are reductions in sulfate, elemental carbon, and organic carbon, and increases in fine soil during the spring (March-May) at select sites. These results can be explained by population growth, land-use changes, and improved source controls.

  10. Chemical Composition and Dynamics of the Upper Troposphere and the Lower Stratosphere: Overview of the Project

    NASA Astrophysics Data System (ADS)

    Sofieva, V. F.; Liu, C.; Huang, F.; Kyrola, E.; Liu, Y.; Ialongo, I.; Hakkarainen, J.; Zhang, Y.

    2016-08-01

    The DRAGON-3 cooperation study on the upper troposphere and the lower stratosphere (UTLS) is based on new satellite data and modern atmospheric models. The objectives of the project are: (i) assessment of satellite data on chemical composition in UTLS, (ii) dynamical and chemical structures of the UTLS and its variability, (iii) multi-scale variability of stratospheric ozone, (iv) climatology of the stratospheric aerosol layer and its variability, and (v) updated ozone climatology and its relation to tropopause/multiple tropopauses.In this paper, we present the main results of the project.

  11. Impacts of increasing the aerosol complexity in the Met Office global numerical weather prediction model

    NASA Astrophysics Data System (ADS)

    Mulcahy, J. P.; Walters, D. N.; Bellouin, N.; Milton, S. F.

    2014-05-01

    The inclusion of the direct and indirect radiative effects of aerosols in high-resolution global numerical weather prediction (NWP) models is being increasingly recognised as important for the improved accuracy of short-range weather forecasts. In this study the impacts of increasing the aerosol complexity in the global NWP configuration of the Met Office Unified Model (MetUM) are investigated. A hierarchy of aerosol representations are evaluated including three-dimensional monthly mean speciated aerosol climatologies, fully prognostic aerosols modelled using the CLASSIC aerosol scheme and finally, initialised aerosols using assimilated aerosol fields from the GEMS project. The prognostic aerosol schemes are better able to predict the temporal and spatial variation of atmospheric aerosol optical depth, which is particularly important in cases of large sporadic aerosol events such as large dust storms or forest fires. Including the direct effect of aerosols improves model biases in outgoing long-wave radiation over West Africa due to a better representation of dust. However, uncertainties in dust optical properties propagate to its direct effect and the subsequent model response. Inclusion of the indirect aerosol effects improves surface radiation biases at the North Slope of Alaska ARM site due to lower cloud amounts in high-latitude clean-air regions. This leads to improved temperature and height forecasts in this region. Impacts on the global mean model precipitation and large-scale circulation fields were found to be generally small in the short-range forecasts. However, the indirect aerosol effect leads to a strengthening of the low-level monsoon flow over the Arabian Sea and Bay of Bengal and an increase in precipitation over Southeast Asia. Regional impacts on the African Easterly Jet (AEJ) are also presented with the large dust loading in the aerosol climatology enhancing of the heat low over West Africa and weakening the AEJ. This study highlights the

  12. Aerosol typing - key information from aerosol studies

    NASA Astrophysics Data System (ADS)

    Mona, Lucia; Kahn, Ralph; Papagiannopoulos, Nikolaos; Holzer-Popp, Thomas; Pappalardo, Gelsomina

    2016-04-01

    Aerosol typing is a key source of aerosol information from ground-based and satellite-borne instruments. Depending on the specific measurement technique, aerosol typing can be used as input for retrievals or represents an output for other applications. Typically aerosol retrievals require some a priori or external aerosol type information. The accuracy of the derived aerosol products strongly depends on the reliability of these assumptions. Different sensors can make use of different aerosol type inputs. A critical review and harmonization of these procedures could significantly reduce related uncertainties. On the other hand, satellite measurements in recent years are providing valuable information about the global distribution of aerosol types, showing for example the main source regions and typical transport paths. Climatological studies of aerosol load at global and regional scales often rely on inferred aerosol type. There is still a high degree of inhomogeneity among satellite aerosol typing schemes, which makes the use different sensor datasets in a consistent way difficult. Knowledge of the 4d aerosol type distribution at these scales is essential for understanding the impact of different aerosol sources on climate, precipitation and air quality. All this information is needed for planning upcoming aerosol emissions policies. The exchange of expertise and the communication among satellite and ground-based measurement communities is fundamental for improving long-term dataset consistency, and for reducing aerosol type distribution uncertainties. Aerosol typing has been recognized as one of its high-priority activities of the AEROSAT (International Satellite Aerosol Science Network, http://aero-sat.org/) initiative. In the AEROSAT framework, a first critical review of aerosol typing procedures has been carried out. The review underlines the high heterogeneity in many aspects: approach, nomenclature, assumed number of components and parameters used for the

  13. The Version 2 Global Precipitation Climatology Project (GPCP) Monthly Precipitation Analysis (1979-Present)

    NASA Technical Reports Server (NTRS)

    Adler, Robert F.; Huffman, George J.; Chang, Alfred; Ferraro, Ralph; Xie, Ping-Ping; Janowiak, John; Rudolf, Bruno; Schneider, Udo; Curtis, Scott; Bolvin, David

    2003-01-01

    The Global Precipitation Climatology Project (GPCP) Version 2 Monthly Precipitation Analysis is described. This globally complete, monthly analysis of surface precipitation at 2.5 degrees x 2.5 degrees latitude-longitude resolution is available from January 1979 to the present. It is a merged analysis that incorporates precipitation estimates from low-orbit-satellite microwave data, geosynchronous-orbit-satellite infrared data, and rain gauge observations. The merging approach utilizes the higher accuracy of the low-orbit microwave observations to calibrate, or adjust, the more frequent geosynchronous infrared observations. The data set is extended back into the premicrowave era (before 1987) by using infrared-only observations calibrated to the microwave-based analysis of the later years. The combined satellite-based product is adjusted by the raingauge analysis. This monthly analysis is the foundation for the GPCP suite of products including those at finer temporal resolution, satellite estimate, and error estimates for each field. The 23-year GPCP climatology is characterized, along with time and space variations of precipitation.

  14. The first ISLSCP field experiment (FIFE). [International Satellite Land Surface Climatology Project

    NASA Technical Reports Server (NTRS)

    Sellers, P. J.; Hall, F. G.; Asrar, G.; Strebel, D. E.; Murphy, R. E.

    1988-01-01

    The background and planning of the first International Satellite Land Surface Climatology Project (ISLSCP) field experiment (FIFE) are discussed. In FIFE, the NOAA series of satellites and GOES will be used to provide a moderate-temporal resolution coarse-spatial resolution data set, with SPOT and aircraft data providing the high-spatial resolution pointable-instrument capability. The paper describes the experiment design, the measurement strategy, the configuration of the site of the experiment (which will be at and around the Konza prairie near Manhattan, Kansas), and the experiment's operations and execution.

  15. Aerosol Retrievals Using Channel 1 and 2 AVHRR Data

    NASA Technical Reports Server (NTRS)

    Mishchenko, Michael I.; Geogdzhayev, Igor V.; Cairns, Brian; Rossow, William B.

    1999-01-01

    The effect of tropospheric aerosols on global climate via the direct and indirect radiative forcings is one of the largest remaining uncertainties in climate change studies. Current assessments of the direct aerosol radiative effect mainly focus on sulfate aerosols. It has become clear, however, that other aerosol types like soil dust and smoke from biomass burning are also likely to be important climate forcing factors. The magnitude and even the sign of the climate forcing caused by these aerosol types is still unknown. General circulation models (GCMs) can be used to estimate the climatic effect of the direct radiative forcing by tropospheric and stratospheric aerosols. Aerosol optical properties are already parameterized in the Goddard Institute for Space Studies GCM. Once the global distribution of aerosol properties (optical thickness, size distribution, and chemical composition) is available, the calculation of the direct aerosol forcing is rather straighfforward. However, estimates of the indirect aerosol effect require additional knowledge of the physics and chemistry of aerosol-cloud interactions which are still poorly understood. One of the main objectives of the Global Aerosol Climatology Project, established in 1998 as a joint initiative of NASA's Radiation Science Program and GEWEX, is to infer the global distribution of aerosols, their properties, and their seasonal and interannual variations for the full period of available satellite data. This will be accomplished primarily through a systematic application of multichannel aerosol retrieval algorithms to existing satellite data and advanced 3-dimensional aerosol chemistry/transport models. In this paper we outline the methodology of analyzing channel 1 and 2 AVHRR radiance data over the oceans and describe preliminary retrieval results.

  16. Aerosol layer height from synergistic use of VIIRS and OMPS

    NASA Astrophysics Data System (ADS)

    Lee, J.; Hsu, N. Y. C.; Sayer, A. M.; Kim, W.; Seftor, C. J.

    2017-12-01

    This study presents an Aerosol Single-scattering albedo and Height Estimation (ASHE) algorithm, which retrieves the height of UV-absorbing aerosols by synergistically using the Visible Infrared Imaging Radiometer Suite (VIIRS) and the Ozone Mapping and Profiler Suite (OMPS). ASHE provides height information over a much broader area than ground-based or spaceborne lidar measurements by benefitting from the wide swaths of the two instruments used. As determination of single-scattering albedo (SSA) of the aerosol layer is the most critical part for the performance and coverage of ASHE, here we demonstrate three different strategies to constrain the SSA. First, ASHE is able to retrieve the SSA of UV-absorbing aerosols when Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) provides vertical profiles of the aerosol layer of interest. Second, Aerosol Robotic Network (AERONET) inversions can directly constrain the SSA of the aerosol layer when collocated with VIIRS or OMPS. Last, a SSA climatology from ASHE, AERONET, or other data sources can be used for large-scale, aged aerosol events, for which climatological SSA is well-known, at the cost of a slight decrease in retrieval accuracy. The same algorithm can be applied to measurements of similar type, such as those made by the Moderate Resolution Imaging Spectroradiometer (MODIS) and Ozone Monitoring Instrument (OMI), for a long-term, consistent data record.

  17. Constructing An Event Based Aerosol Product Under High Aerosol Loading Conditions

    NASA Astrophysics Data System (ADS)

    Levy, R. C.; Shi, Y.; Mattoo, S.; Remer, L. A.; Zhang, J.

    2016-12-01

    High aerosol loading events, such as the Indonesia's forest fire in Fall 2015 or the persistent wintertime haze near Beijing, gain tremendous interests due to their large impact on regional visibility and air quality. Understanding the optical properties of these events and further being able to simulate and predict these events are beneficial. However, it is a great challenge to consistently identify and then retrieve aerosol optical depth (AOD) from passive sensors during heavy aerosol events. Some reasons include:1). large differences between optical properties of high-loading aerosols and those under normal conditions, 2) spectral signals of optically thick aerosols can be mistaken with surface depending on aerosol types, and 3) Extremely optically thick aerosol plumes can also be misidentified as clouds due to its high optical thickness. Thus, even under clear-sky conditions, the global distribution of extreme aerosol events is not well captured in datasets such as the MODIS Dark-Target (DT) aerosol product. In this study, with the synthetic use of OMI Aerosol Index, MODIS cloud product, and operational DT product, the heavy smoke events over the seven sea region are identified and retrieved over the dry season. An event based aerosol product that would compensate the standard "global" aerosol retrieval will be created and evaluated. The impact of missing high AOD retrievals on the regional aerosol climatology will be studied using this newly developed research product.

  18. An A-Train Climatology of Extratropical Cyclone Clouds

    NASA Technical Reports Server (NTRS)

    Posselt, Derek J.; van den Heever, Susan C.; Booth, James F.; Del Genio, Anthony D.; Kahn, Brian; Bauer, Mike

    2016-01-01

    Extratropical cyclones (ETCs) are the main purveyors of precipitation in the mid-latitudes, especially in winter, and have a significant radiative impact through the clouds they generate. However, general circulation models (GCMs) have trouble representing precipitation and clouds in ETCs, and this might partly explain why current GCMs disagree on to the evolution of these systems in a warming climate. Collectively, the A-train observations of MODIS, CloudSat, CALIPSO, AIRS and AMSR-E have given us a unique perspective on ETCs: over the past 10 years these observations have allowed us to construct a climatology of clouds and precipitation associated with these storms. This has proved very useful for model evaluation as well in studies aimed at improving understanding of moist processes in these dynamically active conditions. Using the A-train observational suite and an objective cyclone and front identification algorithm we have constructed cyclone centric datasets that consist of an observation-based characterization of clouds and precipitation in ETCs and their sensitivity to large scale environments. In this presentation, we will summarize the advances in our knowledge of the climatological properties of cloud and precipitation in ETCs acquired with this unique dataset. In particular, we will present what we have learned about southern ocean ETCs, for which the A-train observations have filled a gap in this data sparse region. In addition, CloudSat and CALIPSO have for the first time provided information on the vertical distribution of clouds in ETCs and across warm and cold fronts. We will also discuss how these observations have helped identify key areas for improvement in moist processes in recent GCMs. Recently, we have begun to explore the interaction between aerosol and cloud cover in ETCs using MODIS, CloudSat and CALIPSO. We will show how aerosols are climatologically distributed within northern hemisphere ETCs, and how this relates to cloud cover.

  19. The Two-Column Aerosol Project: Phase I - Overview and Impact of Elevated Aerosol Layers on Aerosol Optical Depth

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Berg, Larry K.; Fast, Jerome D.; Barnard, James C.

    2016-01-08

    The Two-Column Aerosol Project (TCAP), which was conducted from June 2012 through June 2013, was a unique field study that was designed to provide a comprehensive data set that can be used to investigate a number of important climate science questions, including those related to aerosol mixing state and aerosol radiative forcing. The study was designed to sample the atmosphere at a number of altitudes, from near the surface to as high as 8 km, within two atmospheric columns; one located near the coast of North America (over Cape Cod, MA) and a second over the Atlantic Ocean several hundredmore » kilometers from the coast. TCAP included the yearlong deployment of the U.S. Department of Energy’s (DOE) Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) that was located at the base of the Cape Cod column, as well as summer and winter aircraft intensive observation periods of the ARM Aerial Facility. One important finding from TCAP is the relatively common occurrence (on four of six nearly cloud-free flights) of elevated aerosol layers in both the Cape Cod and maritime columns that were detected using the nadir pointing second-generation NASA high-spectral resolution lidar (HSRL-2). These layers contributed up to 60% of the total aerosol optical depth (AOD) observed in the column. Many of these layers were also intercepted by the aircraft configured for in situ sampling, and the aerosol in the layers was found to have increased amounts of biomass burning aerosol and nitrate compared to the aerosol found near the surface.« less

  20. The Two-Column Aerosol Project: Phase I-Overview and impact of elevated aerosol layers on aerosol optical depth

    DOE PAGES

    Berg, Larry K.; Fast, Jerome D.; Barnard, James C.; ...

    2016-01-08

    The Two-Column Aerosol Project (TCAP), conducted from June 2012 through June 2013, was a unique study designed to provide a comprehensive data set that can be used to investigate a number of important climate science questions, including those related to aerosol mixing state and aerosol radiative forcing. The study was designed to sample the atmosphere between and within two atmospheric columns; one fixed near the coast of North America (over Cape Cod, MA) and a second moveable column over the Atlantic Ocean several hundred kilometers from the coast. The U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) Mobile Facilitymore » (AMF) was deployed at the base of the Cape Cod column, and the ARM Aerial Facility was utilized for the summer and winter intensive observation periods. One important finding from TCAP is that four of six nearly cloud-free flight days had aerosol layers aloft in both the Cape Cod and maritime columns that were detected using the nadir pointing second-generation NASA high-spectral resolution lidar (HSRL-2). In addition, these layers contributed up to 60% of the total observed aerosol optical depth (AOD). Many of these layers were also intercepted by the aircraft configured for in situ sampling, and the aerosol in the layers was found to have increased amounts of biomass burning material and nitrate compared to aerosol found near the surface. Lastly, while there was a great deal of spatial and day-to-day variability in the aerosol chemical composition and optical properties, no systematic differences between the two columns were observed.« less

  1. The Two-Column Aerosol Project: Phase I - Overview and Impact of Elevated Aerosol Layers on Aerosol Optical Depth

    NASA Technical Reports Server (NTRS)

    Berg, Larry K.; Fast, Jerome D.; Barnard, James C.; Burton, Sharon P.; Cairns, Brian; Chand, Duli; Comstock, Jennifer M.; Dunagan, Stephen; Ferrare, Richard A.; Flynn, Connor J.; hide

    2015-01-01

    The Two-Column Aerosol Project (TCAP), conducted from June 2012 through June 2013, was a unique study designed to provide a comprehensive data set that can be used to investigate a number of important climate science questions, including those related to aerosol mixing state and aerosol radiative forcing. The study was designed to sample the atmosphere be tween and within two atmospheric columns; one fixed near the coast of North America (over Cape Cod, MA) and a second moveable column over the Atlantic Ocean several hundred kilometers from the coast. The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) was deployed at the base of the Cape Cod column, and the ARM Aerial Facility was utilized for the summer and winter intensive observation periods. One important finding from TCAP is that four of six nearly cloud-free flight days had aerosol layers aloft in both the Cape Cod and maritime columns that were detected using the nadir pointing second-generation NASA high-spectral resolution lidar (HSRL-2).These layer s contributed up to 60 of the total observed aerosol optical depth (AOD). Many of these layers were also intercepted by the aircraft configured for in situ sampling, and the aerosol in the layers was found to have increased amounts of biomass burning material and nitrate compared to aerosol found near the surface. In addition, while there was a great deal of spatial and day-to-day variability in the aerosol chemical composition and optical properties, no systematic differences between the two columns were observed.

  2. The Two-Column Aerosol Project: Phase I—Overview and impact of elevated aerosol layers on aerosol optical depth

    NASA Astrophysics Data System (ADS)

    Berg, Larry K.; Fast, Jerome D.; Barnard, James C.; Burton, Sharon P.; Cairns, Brian; Chand, Duli; Comstock, Jennifer M.; Dunagan, Stephen; Ferrare, Richard A.; Flynn, Connor J.; Hair, Johnathan W.; Hostetler, Chris A.; Hubbe, John; Jefferson, Anne; Johnson, Roy; Kassianov, Evgueni I.; Kluzek, Celine D.; Kollias, Pavlos; Lamer, Katia; Lantz, Kathleen; Mei, Fan; Miller, Mark A.; Michalsky, Joseph; Ortega, Ivan; Pekour, Mikhail; Rogers, Ray R.; Russell, Philip B.; Redemann, Jens; Sedlacek, Arthur J.; Segal-Rosenheimer, Michal; Schmid, Beat; Shilling, John E.; Shinozuka, Yohei; Springston, Stephen R.; Tomlinson, Jason M.; Tyrrell, Megan; Wilson, Jacqueline M.; Volkamer, Rainer; Zelenyuk, Alla; Berkowitz, Carl M.

    2016-01-01

    The Two-Column Aerosol Project (TCAP), conducted from June 2012 through June 2013, was a unique study designed to provide a comprehensive data set that can be used to investigate a number of important climate science questions, including those related to aerosol mixing state and aerosol radiative forcing. The study was designed to sample the atmosphere between and within two atmospheric columns; one fixed near the coast of North America (over Cape Cod, MA) and a second moveable column over the Atlantic Ocean several hundred kilometers from the coast. The U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) was deployed at the base of the Cape Cod column, and the ARM Aerial Facility was utilized for the summer and winter intensive observation periods. One important finding from TCAP is that four of six nearly cloud-free flight days had aerosol layers aloft in both the Cape Cod and maritime columns that were detected using the nadir pointing second-generation NASA high-spectral resolution lidar (HSRL-2). These layers contributed up to 60% of the total observed aerosol optical depth (AOD). Many of these layers were also intercepted by the aircraft configured for in situ sampling, and the aerosol in the layers was found to have increased amounts of biomass burning material and nitrate compared to aerosol found near the surface. In addition, while there was a great deal of spatial and day-to-day variability in the aerosol chemical composition and optical properties, no systematic differences between the two columns were observed.

  3. Estimation of polar stratospheric cloud infrared extinction climatology using visible satellite observations

    NASA Technical Reports Server (NTRS)

    Pitts, Michael C.; Thomason, Larry W.

    1995-01-01

    Polar stratospheric clouds (PSC's) provide surfaces for heterogeneous processes which can dramatically alter the normal partitioning of odd nitrogen and chlorine families in the winter polar stratospheres, setting up conditions for significant ozone depletion as manifested in the springtime Antarctic ozone hole. The spatial and temporal distribution of PSC's is important for parameterizing PSC occurrence in multidimensional photochemical models whose use is essential for fully understanding observed Antarctic ozone losses as well as for accessing the possibility of a similar phemonenon occurring in the future in the Arctic. The Stratospheric Aerosol Measurement (SAM) 2 sensor, a single-channel (1mu m) photometer launched into a Sun-synchronous orbit aboard the Nimbus 7 satellite in October 1978, provided a unique database to establish the climatology of PSC's. Poole and Pitts (1994) used the record of high-latitude aerosol extinction obtained by SAM II from 1979-1989 to establish the climatology of PSC occurrences in the Arctic and Antarctic. Unfortunately, little information about PSC composition or type was detectable from the single-wavelength SAM II data.

  4. The SHADOZ Data Base: History, Archive Web Guide, and Sample Climatologies

    NASA Technical Reports Server (NTRS)

    White, J. C.; Thompson, A. M.; Einaudi, Franco (Technical Monitor)

    2000-01-01

    SHADOZ (Southern Hemisphere Additional Ozonesonde) is a project to augment and archive ozonesonde data from ten tropical and subtropical ozone stations. Started in 1998 by NASA's Goddard Space Flight Center and other US and international co-investigators, SHADOZ is an important tool for tropospheric ozone research in the equatorial region. The rationale for SHADOZ is to: (1) validate and improve remote sensing techniques (e.g., the Total Ozone Mapping Spectrometer (TOMS) satellite) for estimating tropical ozone, (2) contribute to climatology and trend analyses of tropical ozone and (3) provide research topics to scientists and educate students, especially in participating countries. SHADOZ is envisioned as a data service to the global scientific community by providing a central public archive location via the internet: http://code9l6.gsfc.nasa.gov/Data_services/shadoz. While the SHADOZ website maintains a standard data format for the archive, it also informs the data users on the differing stations' preparation techniques and data treatment. The presentation navigates through the SHADOZ website to access each station's sounding data and summarize each station's characteristics. Since the start of the project in 1998, the SHADOZ archive has accumulated over 600 ozonesonde profiles and received over 30,000 outside data requests. Data also includes launches from various SHADOZ supported field campaigns, such as, the Indian Ocean Experiment (INDOEX), Sounding of Ozone and Water in the Equatorial Region (SOWER) and Aerosols99 Atlantic Cruise. Using data from the archive, sample climatologies and profiles from selected stations and campaigns will be shown.

  5. Improved Gridded Aerosol Data for India

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Gueymard, C.; Sengupta, M.

    Using point data from ground sites in and around India equipped with multiwavelength sunphotometers, as well as gridded data from space measurements or from existing aerosol climatologies, an improved gridded database providing the monthly aerosol optical depth at 550 nm (AOD550) and Angstrom exponent (AE) over India is produced. Data from 83 sunphotometer sites are used here as ground truth tocalibrate, optimally combine, and validate monthly gridded data during the period from 2000 to 2012.

  6. Future projections of temperature and precipitation climatology for CORDEX-MENA domain using RegCM4.4

    NASA Astrophysics Data System (ADS)

    Ozturk, Tugba; Turp, M. Tufan; Türkeş, Murat; Kurnaz, M. Levent

    2018-07-01

    In this study, we investigate changes in seasonal temperature and precipitation climatology of CORDEX Middle East and North Africa (MENA) region for three periods of 2010-2040, 2040-2070 and 2070-2100 with respect to the control period of 1970-2000 by using regional climate model simulations. Projections of future climate conditions are modeled by forcing Regional Climate Model, RegCM4.4 of the International Centre for Theoretical Physics (ICTP) with two different CMIP5 global climate models. HadGEM2-ES global climate model of the Met Office Hadley Centre and MPI-ESM-MR global climate model of the Max Planck Institute for Meteorology were used to generate 50 km resolution data for the Coordinated Regional Climate Downscaling Experiment (CORDEX) Region 13. We test the seasonal time-scale performance of RegCM4.4 in simulating the observed climatology over domain of the MENA by using the output of two different global climate models. The projection results show relatively high increase of average temperatures from 3 °C up to 9 °C over the domain for far future (2070-2100). A strong decrease in precipitation is projected in almost all parts of the domain according to the output of the regional model forced by scenario outputs of two global models. Therefore, warmer and drier than present climate conditions are projected to occur more intensely over the CORDEX-MENA domain.

  7. High Resolution Hydro-climatological Projections for Western Canada

    NASA Astrophysics Data System (ADS)

    Erler, Andre Richard

    Accurate identification of the impact of global warming on water resources and hydro-climatic extremes represents a significant challenge to the understanding of climate change on the regional scale. Here an analysis of hydro-climatic changes in western Canada is presented, with specific focus on the Fraser and Athabasca River basins and on changes in hydro-climatic extremes. The analysis is based on a suite of simulations designed to characterize internal variability, as well as model uncertainty. A small ensemble of Community Earth System Model version 1 (CESM1) simulations was employed to generate global climate projections, which were downscaled to 10 km resolution using the Weather Research and Forecasting model (WRF V3.4.1) with several sets of physical parameterizations. Downscaling was performed for a historical validation period and a mid- and end-21st-century projection period, using the RCP8.5 greenhouse gas trajectory. Daily station observations and monthly gridded datasets were used for validation. Changes in hydro-climatic extremes are characterized using Extreme Value Analysis. A novel method of aggregating data from climatologically similar stations was employed to increase the statistical power of the analysis. Changes in mean and extreme precipitation are found to differ strongly between seasons and regions, but (relative) changes in extremes generally follow changes in the (seasonal) mean. At the end of the 21st century, precipitation and precipitation extremes are projected to increase by 30% at the coast in fall and land-inwards in winter, while the projected increase in summer precipitation is smaller and changes in extremes are often not statistically significant. Reasons for the differences between seasons, the role of precipitation recycling in atmospheric water transport, and the sensitivity to physics parameterizations are discussed. Major changes are projected for the Fraser River basin, including earlier snowmelt and a 50% reduction in

  8. Comparison between calculations of shortwave radiation with different aerosol datasets and measured data at the MSU MO (Russia)

    NASA Astrophysics Data System (ADS)

    Poliukhov, Aleksei; Chubarova, Natalia; Kinne, Stephan; Rivin, Gdaliy; Shatunova, Marina; Tarasova, Tatiana

    2017-02-01

    The radiation block of the COSMO non-hydrostatic mesoscale model of the atmosphere and soil active layer was tested against a relatively new effective CLIRAD(FC05)-SW radiation model and radiative measurements at the Moscow State University Meteorological Observatory (MSU MO, 55.7N, 37.5E) using different aerosol datasets in cloudless conditions. We used the data of shortwave radiation components from the Kipp&Zonen net radiometer CNR4. The model simulations were performed with the application of various aerosol climatologies including the new MACv2 climatology and the aerosol and water vapor dataset from CIMEL (AERONET) sun photometer measurements. The application of the new MACv2 climatology in the CLIRAD(FC05)-SW radiation model provides the annual average relative error of the total global radiation of -3% varying from 0.5% in May to -7.7% in December. The uncertainty of radiative calculations in the COSMO model according to preliminary estimates changes from 1.4% to 8.4%. against CLIRAD(FC05)-SW radiation model with the same parameters. We showed that in clear sky conditions the sensitivity of air temperature at 2 meters to shortwave net radiation changes is about 0.7-0.9°C per100 W/m2 due to the application of aerosol climatologies over Moscow.

  9. Two-Column Aerosol Project: Aerosol Light Extinction Measurements Field Campaign Report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dubey, Manvendra; Aiken, Allison; Berg, Larry

    We deployed Aerodyne Research Inc.’s first Cavity Attenuated Phase Shift extinction (CAPS PMex) monitor (built by Aerodyne) that measures light extinction by using a visible-light-emitting diode (LED) as a light source, a sample cell incorporating two high-reflectivity mirrors centered at the wavelength of the LED, and a vacuum photodiode detector in Cape Cod in 2012/13 for the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility’s Two-Column Aerosol Project (TCAP). The efficacy of this instrument is based on the fact that aerosols are broadband scatterers and absorbers of light. The input LED is square-wave modulated and passedmore » through the sample cell that distorts it due to exponential decay by aerosol light absorption and scattering; this is measured at the detector. The amount of phase shift of the light at the detector is used to determine the light extinction. This extinction measurement provides an absolute value, requiring no calibration. The goal was to compare the CAPS performance with direct measurements of absorption with ARM’s baseline photoacoustic soot spectrometer (PASS-3) and nephelometer instruments to evaluate its performance.« less

  10. Chemical climatology of the southeastern United States, 1999-2013

    NASA Astrophysics Data System (ADS)

    Hidy, G. M.; Blanchard, C. L.; Baumann, K.; Edgerton, E.; Tanenbaum, S.; Shaw, S.; Knipping, E.; Tombach, I.; Jansen, J.; Walters, J.

    2014-06-01

    A series of experiments (the Southern Oxidant and Aerosol Study-SOAS) took place in central Alabama in June-July 2013 as part of the broader Southern Atmosphere Study (SAS). These projects were aimed at studying oxidant photochemistry and formation and impacts of aerosols at a detailed process level in a location where high biogenic organic vapor emissions interact with anthropogenic emissions, and the atmospheric chemistry occurs in a subtropical climate in North America. The majority of the ground-based experiments were located at the Southeastern Aerosol Research and Characterization (SEARCH) Centreville (CTR) site near Brent, Alabama, where extensive, unique aerometric measurements of meteorology, trace gases and particles have been made from the early 1990s through 2013. The SEARCH network data permits a characterization of temporal and spatial context of the SOAS findings. The long-term measurements show that the SOAS experiments took place during the second wettest and coolest year in the 2000-2013 period, with lower than average solar radiation. The pollution levels at CTR and other SEARCH sites were the lowest since full measurements began in 1999. This dataset provides a perspective for the SOAS program in terms of long-term average chemistry (chemical climatology) and short-term comparisons of summer average spatial variability across the Southeast at high temporal (hourly) resolution. Changes in anthropogenic gas and particle emissions between 1999 and 2013, account for the decline in pollutant concentrations at the monitoring sites in the region. The long-term and short-term data provide an opportunity to contrast SOAS results with temporally and spatially variable conditions in support for the development of tests for the robustness of SOAS findings.

  11. Radiative Effects of Aerosol in the Marine Environment: Tales from the Two-Column Aerosol Project

    NASA Astrophysics Data System (ADS)

    Berg, L. K.; Fast, J. D.; Barnard, J.; Chand, D.; Chapman, E. G.; Comstock, J. M.; Ferrare, R. A.; Flynn, C. J.; Hair, J. W.; Hostetler, C. A.; Hubbe, J.; Johnson, R.; Kassianov, E.; Kluzek, C.; Laskin, A.; Lee, Y.; Mei, F.; Michalsky, J. J.; Redemann, J.; Rogers, R. R.; Russell, P. B.; Sedlacek, A. J.; Schmid, B.; Shilling, J. E.; Shinozuka, Y.; Springston, S. R.; Tomlinson, J. M.; Wilson, J. M.; Zelenyuk, A.; Berkowitz, C. M.

    2013-12-01

    There is still uncertainty associated with the direct radiative forcing by atmospheric aerosol and its representation in atmospheric models. This is particularly true in marine environments near the coast where the aerosol loading is a function of both naturally occurring and anthropogenic aerosol. These regions are also subject to variable synoptic and thermally driven flows (land-sea breezes) that transport aerosol between the continental and marine environments. The situation is made more complicated due to seasonal changes in aerosol emissions. Given these differences in emissions, we expect significant differences in the aerosol intensive and extensive properties between summer and winter and data is needed to evaluate models over the wide range of conditions. To address this issue, the recently completed Two Column Aerosol Project (TCAP) was designed to measure the key aerosol parameters in two atmospheric columns, one located over Cape Cod, Massachusetts and another approximately 200 km from the coast over the Atlantic Ocean. Measurements included aerosol size distribution, chemical composition, optical properties and vertical distribution. Several aspects make TCAP unique, including the year-long deployment of a suite of surface-based instruments by the US Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility and two aircraft intensive operations periods supported by the ARM Airborne Facility, one conducted in July 2012 and a second in February 2013. The presentation will include a discussion of the impact of the aerosol optical properties and their uncertainty on simulations of the radiation budget within the TCAP domain in the context of both single column and regional scale models. Data from TCAP will be used to highlight a number of important factors, including diurnal variation in aerosol optical depth measured at the surface site, systematic changes in aerosol optical properties (including scattering, absorption, and

  12. A 20-year simulated climatology of global dust aerosol deposition.

    PubMed

    Zheng, Yu; Zhao, Tianliang; Che, Huizheng; Liu, Yu; Han, Yongxiang; Liu, Chong; Xiong, Jie; Liu, Jianhui; Zhou, Yike

    2016-07-01

    Based on a 20-year (1991-2010) simulation of dust aerosol deposition with the global climate model CAM5.1 (Community Atmosphere Model, version 5.1), the spatial and temporal variations of dust aerosol deposition were analyzed using climate statistical methods. The results indicated that the annual amount of global dust aerosol deposition was approximately 1161±31Mt, with a decreasing trend, and its interannual variation range of 2.70% over 1991-2010. The 20-year average ratio of global dust dry to wet depositions was 1.12, with interannual variation of 2.24%, showing the quantity of dry deposition of dust aerosol was greater than dust wet deposition. High dry deposition was centered over continental deserts and surrounding regions, while wet deposition was a dominant deposition process over the North Atlantic, North Pacific and northern Indian Ocean. Furthermore, both dry and wet deposition presented a zonal distribution. To examine the regional changes of dust aerosol deposition on land and sea areas, we chose the North Atlantic, Eurasia, northern Indian Ocean, North Pacific and Australia to analyze the interannual and seasonal variations of dust deposition and dry-to-wet deposition ratio. The deposition amounts of each region showed interannual fluctuations with the largest variation range at around 26.96% in the northern Indian Ocean area, followed by the North Pacific (16.47%), Australia (9.76%), North Atlantic (9.43%) and Eurasia (6.03%). The northern Indian Ocean also had the greatest amplitude of interannual variation in dry-to-wet deposition ratio, at 22.41%, followed by the North Atlantic (9.69%), Australia (6.82%), North Pacific (6.31%) and Eurasia (4.36%). Dust aerosol presented a seasonal cycle, with typically strong deposition in spring and summer and weak deposition in autumn and winter. The dust deposition over the northern Indian Ocean exhibited the greatest seasonal change range at about 118.00%, while the North Atlantic showed the lowest seasonal

  13. Background stratospheric aerosol and polar stratospheric cloud reference models

    NASA Technical Reports Server (NTRS)

    Mccormick, M. P.; Wang, P.-H.; Pitts, M. C.

    1993-01-01

    A global aerosol climatology is evolving from the NASA satellite experiments SAM II, SAGE I, and SAGE II. In addition, polar stratospheric cloud (PSC) data have been obtained from these experiments over the last decade. An undated reference model of the optical characteristics of the background aerosol is described and a new aerosol reference model derived from the latest available data is proposed. The aerosol models are referenced to the height above the tropopause. The impact of a number of volcanic eruptions is described. In addition, a model describing the seasonal, longitudinal, and interannual variations in PSCs is presented.

  14. ARTIST: An International Project Investigating Aerosol Retention in a Ruptured Steam Generator

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Guentay, S.; Dehbi, A.; Suckow, D.

    2002-07-01

    Steam generator tube ruptures (SGTR) with a concurrent stuck open safety relief valve are counted among the risk dominant accident sequences because of the potential for radioactive products to bypass the containment. Owing to the absence of relevant empirical data and the complexity of the geometry and controlling processes, the aerosol removal in the steam generator (SG) tubes and in the secondary side is not well understood. Therefore, little or no credit is usually taken for aerosol retention due to natural processes in the various components of a SG. To help reduce the uncertainties associated with fission product release followingmore » an SGTR sequence, the Paul Scherrer Institut has initiated an international experimental project to be performed in the ARTIST (AeRosol Trapping In a Steam generaTor) facility in the time period from 2002 to 2007. The ARTIST test section is a scaled model of a real SG, and is comprised of a 264-tube bundle with a maximum height of 3.8 m, as well as one full-size droplet separator and one full-size steam dryer. The ARTIST facility is capable of producing soluble and insoluble aerosols and entrain them at sonic gas flow rates (up to 0.25 kg/s, thus matching comparable values predicted by the codes. In addition, aerosols can be generated at prototypical concentrations (up to 5 g/m{sup 3}) and sizes (0.2-5 mm AMMD). State of the art instrumentation is used (Low-pressure impactors, photometers, on-line particle sizer, online droplet sizer, etc.). The ARTIST project will simulate the flow and retention of aerosol-borne fission products in the SG, and provide a unique database to support safety assessments and analytical models. The project is foreseen in seven phases: 1) Aerosol retention in the tube under dry secondary side conditions, 2) Aerosol retention in the near field close to break under dry conditions, 3) Aerosol retention in the bundle far field under dry conditions, 4) Aerosol retention in the separator and dryer under

  15. On the representation of aerosol activation and its influence on model-derived estimates of the aerosol indirect effect

    NASA Astrophysics Data System (ADS)

    Rothenberg, Daniel; Avramov, Alexander; Wang, Chien

    2018-06-01

    Interactions between aerosol particles and clouds contribute a great deal of uncertainty to the scientific community's understanding of anthropogenic climate forcing. Aerosol particles serve as the nucleation sites for cloud droplets, establishing a direct linkage between anthropogenic particulate emissions and clouds in the climate system. To resolve this linkage, the community has developed parameterizations of aerosol activation which can be used in global climate models to interactively predict cloud droplet number concentrations (CDNCs). However, different activation schemes can exhibit different sensitivities to aerosol perturbations in different meteorological or pollution regimes. To assess the impact these different sensitivities have on climate forcing, we have coupled three different core activation schemes and variants with the CESM-MARC (two-Moment, Multi-Modal, Mixing-state-resolving Aerosol model for Research of Climate (MARC) coupled with the National Center for Atmospheric Research's (NCAR) Community Earth System Model (CESM; version 1.2)). Although the model produces a reasonable present-day CDNC climatology when compared with observations regardless of the scheme used, ΔCDNCs between the present and preindustrial era regionally increase by over 100 % in zonal mean when using the most sensitive parameterization. These differences in activation sensitivity may lead to a different evolution of the model meteorology, and ultimately to a spread of over 0.8 W m-2 in global average shortwave indirect effect (AIE) diagnosed from the model, a range which is as large as the inter-model spread from the AeroCom intercomparison. Model-derived AIE strongly scales with the simulated preindustrial CDNC burden, and those models with the greatest preindustrial CDNC tend to have the smallest AIE, regardless of their ΔCDNC. This suggests that present-day evaluations of aerosol-climate models may not provide useful constraints on the magnitude of the AIE, which

  16. Aerosol Remote Sensing from AERONET, the Ground-Based Satellite

    NASA Technical Reports Server (NTRS)

    Holben, Brent N.

    2012-01-01

    Atmospheric particles including mineral dust, biomass burning smoke, pollution from carbonaceous aerosols and sulfates, sea salt, impact air quality and climate. The Aerosol Robotic Network (AERONET) program, established in the early 1990s, is a federation of ground-based remote sensing aerosol networks of Sun/sky radiometers distributed around the world, which provides a long-term, continuous and readily accessible public domain database of aerosol optical (e.g., aerosol optical depth) and microphysical (e.g., aerosol volume size distribution) properties for aerosol characterization, validation of satellite retrievals, and synergism with Earth science databases. Climatological aerosol properties will be presented at key worldwide locations exhibiting discrete dominant aerosol types. Further, AERONET's temporary mesoscale network campaign (e.g., UAE2, TIGERZ, DRAGON-USA.) results that attempt to quantify spatial and temporal variability of aerosol properties, establish validation of ground-based aerosol retrievals using aircraft profile measurements, and measure aerosol properties on compatible spatial scales with satellite retrievals and aerosol transport models allowing for more robust validation will be discussed.

  17. Aerosol chemistry in GLOBE

    NASA Technical Reports Server (NTRS)

    Clarke, Antony D.; Rothermel, Jeffry; Jarzembski, Maurice A.

    1993-01-01

    This task addresses the measurement and understanding of the physical and chemical properties of aerosol in remote regions that are responsible for aerosol backscatter at infrared wavelengths. Because it is representative of other clean areas, the remote Pacific is of extreme interest. Emphasis is on the determination size dependent aerosol properties that are required for modeling backscatter at various wavelengths and upon those features that may be used to help understand the nature, origin, cycling and climatology of these aerosols in the remote troposphere. Empirical relationships will be established between lidar measurements and backscatter derived from the aerosol microphysics as required by the NASA Doppler Lidar Program. This will include the analysis of results from the NASA GLOBE Survey Mission Flight Program. Additional instrument development and deployment will be carried out in order to extend and refine this data base. Identified activities include participation in groundbased and airborne experiments. Progress to date includes participation in, analysis of, and publication of results from Mauna Loa Backscatter Intercomparison Experiment (MABIE) and Global Backscatter Experiment (GLOBE).

  18. Chemical climatology of the southeastern United States, 1999-2013

    NASA Astrophysics Data System (ADS)

    Hidy, G. M.; Blanchard, C. L.; Baumann, K.; Edgerton, E.; Tanenbaum, S.; Shaw, S.; Knipping, E.; Tombach, I.; Jansen, J.; Walters, J.

    2014-11-01

    A series of experiments (the Southern Oxidant and Aerosol Study - SOAS) took place in central Alabama in June-July, 2013 as part of the broader Southern Atmosphere Study (SAS). These projects were aimed at studying oxidant photochemistry and formation and impacts of aerosols at a detailed process level in a location where high biogenic organic vapor emissions interact with anthropogenic emissions, and the atmospheric chemistry occurs in a subtropical climate in North America. The majority of the ground-based experiments were located at the Southeastern Aerosol Research and Characterization (SEARCH) Centreville (CTR) site near Brent, Alabama, where extensive, unique aerometric measurements of trace gases and particles and meteorology were made beginning in the early 1990s through 2013. The SEARCH network data permits a characterization of the temporal and spatial context of the SOAS findings. Our earlier analyses of emissions and air quality trends are extended through 2013 to provide a perspective for continued decline in ambient concentrations, and the implications of these changes to regional sulfur oxide, nitrogen-ozone, and carbon chemistry. The narrative supports the SAS program in terms of long-term average chemistry (chemical climatology) and short-term comparisons of early summer average spatial variability across the southeastern US at high temporal (hourly) resolution. The long-term measurements show that the SOAS experiments took place during the second wettest and coolest year in the 2000-2013 period, with lower than average solar radiation. The pollution levels at CTR and other SEARCH sites were the lowest since full measurements began in 1999. Changes in anthropogenic gas and particle emissions between 1999 and 2013 account for the decline in pollutant concentrations at the monitoring sites in the region. The data provide an opportunity to contrast SOAS results with temporally and spatially variable conditions in support of the development of tests

  19. Enviro-HIRLAM/ HARMONIE Studies in ECMWF HPC EnviroAerosols Project

    NASA Astrophysics Data System (ADS)

    Hansen Sass, Bent; Mahura, Alexander; Nuterman, Roman; Baklanov, Alexander; Palamarchuk, Julia; Ivanov, Serguei; Pagh Nielsen, Kristian; Penenko, Alexey; Edvardsson, Nellie; Stysiak, Aleksander Andrzej; Bostanbekov, Kairat; Amstrup, Bjarne; Yang, Xiaohua; Ruban, Igor; Bergen Jensen, Marina; Penenko, Vladimir; Nurseitov, Daniyar; Zakarin, Edige

    2017-04-01

    The EnviroAerosols on ECMWF HPC project (2015-2017) "Enviro-HIRLAM/ HARMONIE model research and development for online integrated meteorology-chemistry-aerosols feedbacks and interactions in weather and atmospheric composition forecasting" is aimed at analysis of importance of the meteorology-chemistry/aerosols interactions and to provide a way for development of efficient techniques for on-line coupling of numerical weather prediction and atmospheric chemical transport via process-oriented parameterizations and feedback algorithms, which will improve both the numerical weather prediction and atmospheric composition forecasts. Two main application areas of the on-line integrated modelling are considered: (i) improved numerical weather prediction with short-term feedbacks of aerosols and chemistry on formation and development of meteorological variables, and (ii) improved atmospheric composition forecasting with on-line integrated meteorological forecast and two-way feedbacks between aerosols/chemistry and meteorology. During 2015-2016 several research projects were realized. At first, the study on "On-line Meteorology-Chemistry/Aerosols Modelling and Integration for Risk Assessment: Case Studies" focused on assessment of scenarios with accidental and continuous emissions of sulphur dioxide for case studies for Atyrau (Kazakhstan) near the northern part of the Caspian Sea and metallurgical enterprises on the Kola Peninsula (Russia), with GIS integration of modelling results into the RANDOM (Risk Assessment of Nature Detriment due to Oil spill Migration) system. At second, the studies on "The sensitivity of precipitation simulations to the soot aerosol presence" & "The precipitation forecast sensitivity to data assimilation on a very high resolution domain" focused on sensitivity and changes in precipitation life-cycle under black carbon polluted conditions over Scandinavia. At third, studies on "Aerosol effects over China investigated with a high resolution

  20. Climatological aspects of aerosol physical characteristics in Tunisia deduced from sun photometric measurements.

    PubMed

    Chaâbane, Mabrouk; Azri, Chafai; Medhioub, Khaled

    2012-01-01

    Atmospheric and climatic data measured at Thala site (Tunisia) for a long-time period (1977-2001) are used to analyse the monthly, seasonal, and annual variations of the aerosol optical depth at 1 μm wavelength. We have shown that aerosol and microphysical properties and the dominating aerosol types depend on seasons. A comparison of the seasonal cycle of aerosol optical characteristics at Thala site showed that the contribution of long-range transported particles is expected to be larger in summer as a consequence of the weather stability typical of this season. Also, the winter decrease in atmospheric turbidity may result from increases in relative humidity and decreases in temperature, leading to increased particle size and mass and increased fall and deposition velocities. The spring and autumn weather patterns usually carry fine dust and sand particles for the desert area to Thala region. The annual behaviour of the aerosol optical depth recorded a period of stead increase started in 1986 until 2001. Trends in atmospheric turbidity after 1988 could be explained other ways by the contribution of the eruption of Mount Pinatubo in 1991 and by local or regional changes in climate or in aerosol emissions.

  1. Climatological simulations of ozone and atmospheric aerosols in the Greater Cairo region

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Steiner, A. L.; Tawfik, A. B.; Shalaby, A.

    An integrated chemistry-climate model (RegCM4-CHEM) simulates present-day climate, ozone and tropospheric aerosols over Egypt with a focus on Greater Cairo (GC) region. The densley populated GC region is known for its severe air quality issues driven by high levels of anthropogenic pollution in conjuction with natural sources such as dust and agricultural burning events. We find that current global emission inventories underestimate key pollutants such as nitrogen oxides and anthropogenic aerosol species. In the GC region, average-ground-based NO2 observations of 40-60 ppb are substantially higher than modeled estimates (5-10 ppb), likely due to model grid resolution, improper boundary layer representation,more » and poor emissions inventories. Observed ozone concentrations range from 35 ppb (winter) to 80 ppb (summer). The model reproduces the seasonal cycle fairly well, but modeled summer ozone is understimated by approximately 15 ppb and exhibits little interannual variability. For aerosols, springtime dust events dominate the seasonal aerosol cycle. The chemistry-climate model captures the springtime peak aerosol optical depth (AOD) of 0.7-1 but is slightly greater than satellite-derived AOD. Observed AOD decreases in the summer and increases again in the fall due to agricultural burning events in the Nile Delta, yet the model underestimates this fall observed AOD peak, as standard emissions inventories underestimate this burning and the resulting aerosol emissions. Our comparison of modeled gas and particulate phase atmospheric chemistry in the GC region indicates that improved emissions inventories of mobile sources and other anthropogenic activities are needed to improve air quality simulations in this region.« less

  2. International Workshop on Stratospheric Aerosols: Measurements, Properties, and Effects

    NASA Technical Reports Server (NTRS)

    Pueschel, Rudolf F. (Editor)

    1991-01-01

    Following a mandate by the International Aerosol Climatology Program under the auspices of International Association of Meteorology and Atmospheric Physics International Radiation Commission, 45 scientists from five nations convened to discuss relevant issues associated with the measurement, properties, and effects of stratospheric aerosols. A summary is presented of the discussions on formation and evolution, transport and fate, effects on climate, role in heterogeneous chemistry, and validation of lidar and satellite remote sensing of stratospheric aerosols. Measurements are recommended of the natural (background) and the volcanically enhanced aerosol (sulfuric acid and silica particles), the exhaust of shuttle, civil aviation and supersonic aircraft operations (alumina, soot, and ice particles), and polar stratospheric clouds (ice, condensed nitric and hydrochloric acids).

  3. Sensitivity of Boreal-Summer Circulation and Precipitation to Atmospheric Aerosols in Selected Regions. Part 2; The Americas

    NASA Technical Reports Server (NTRS)

    Wilcox, E. M.; Sud, Y. C.; Walker, G.

    2009-01-01

    Aerosol perturbations over selected land regions are imposed in Version-4 of the Goddard Earth Observing System (GEOS-4) general circulation model (GCM) to assess the influence of increasing aerosol concentrations on regional circulation patterns and precipitation in four selected regions: India, Africa, and North and South America. Part 1 of this paper addresses the responses to aerosol perturbations in India and Africa. This paper presents the same for aerosol perturbations over the Americas. GEOS-4 is forced with prescribed aerosols based on climatological data, which interact with clouds using a prognostic scheme for cloud microphysics including aerosol nucleation of water and ice cloud hydrometeors. In clear-sky conditions the aerosols interact with radiation. Thus the model includes comprehensive physics describing the aerosol direct and indirect effects on climate (hereafter ADE and AIE respectively). Each simulation is started from analyzed initial conditions for 1 May and was integrated through June-July-August of each of the six years: 1982 1987 to provide a 6-ensemble set. Results are presented for the difference between simulations with double the climatological aerosol concentration and one-half the climatological aerosol concentration for three experiments: two where the ADE and AIE are applied separately and one in which both the ADE and AIE are applied. The ADE and AIE both yield reductions in net radiation at the top of the atmosphere and surface while the direct absorption of shortwave radiation contributes a net radiative heating in the atmosphere. A large net heating of the atmosphere is also apparent over the subtropical North Atlantic Ocean that is attributable to the large aerosol perturbation imposed over Africa. This atmospheric warming and the depression of the surface pressure over North America contribute to a northward shift of the inter-Tropical Convergence Zone over northern America, an increase in precipitation over Central America

  4. Climatological Aspects of Aerosol Physical Characteristics in Tunisia Deduced from Sun Photometric Measurements

    PubMed Central

    Chaâbane, Mabrouk; Azri, Chafai; Medhioub, Khaled

    2012-01-01

    Atmospheric and climatic data measured at Thala site (Tunisia) for a long-time period (1977–2001) are used to analyse the monthly, seasonal, and annual variations of the aerosol optical depth at 1 μm wavelength. We have shown that aerosol and microphysical properties and the dominating aerosol types depend on seasons. A comparison of the seasonal cycle of aerosol optical characteristics at Thala site showed that the contribution of long-range transported particles is expected to be larger in summer as a consequence of the weather stability typical of this season. Also, the winter decrease in atmospheric turbidity may result from increases in relative humidity and decreases in temperature, leading to increased particle size and mass and increased fall and deposition velocities. The spring and autumn weather patterns usually carry fine dust and sand particles for the desert area to Thala region. The annual behaviour of the aerosol optical depth recorded a period of stead increase started in 1986 until 2001. Trends in atmospheric turbidity after 1988 could be explained other ways by the contribution of the eruption of Mount Pinatubo in 1991 and by local or regional changes in climate or in aerosol emissions. PMID:22629150

  5. The NEWS Water Cycle Climatology

    NASA Astrophysics Data System (ADS)

    Rodell, M.; Beaudoing, H. K.; L'Ecuyer, T.; Olson, W. S.

    2012-12-01

    NASA's Energy and Water Cycle Study (NEWS) program fosters collaborative research towards improved quantification and prediction of water and energy cycle consequences of climate change. In order to measure change, it is first necessary to describe current conditions. The goal of the first phase of the NEWS Water and Energy Cycle Climatology project was to develop "state of the global water cycle" and "state of the global energy cycle" assessments based on data from modern ground and space based observing systems and data integrating models. The project was a multi-institutional collaboration with more than 20 active contributors. This presentation will describe the results of the water cycle component of the first phase of the project, which include seasonal (monthly) climatologies of water fluxes over land, ocean, and atmosphere at continental and ocean basin scales. The requirement of closure of the water budget (i.e., mass conservation) at various scales was exploited to constrain the flux estimates via an optimization approach that will also be described. Further, error assessments were included with the input datasets, and we examine these in relation to inferred uncertainty in the optimized flux estimates in order to gauge our current ability to close the water budget within an expected uncertainty range.

  6. The NEWS Water Cycle Climatology

    NASA Technical Reports Server (NTRS)

    Rodell, Matthew; Beaudoing, Hiroko Kato; L'Ecuyer, Tristan; William, Olson

    2012-01-01

    NASA's Energy and Water Cycle Study (NEWS) program fosters collaborative research towards improved quantification and prediction of water and energy cycle consequences of climate change. In order to measure change, it is first necessary to describe current conditions. The goal of the first phase of the NEWS Water and Energy Cycle Climatology project was to develop "state of the global water cycle" and "state of the global energy cycle" assessments based on data from modern ground and space based observing systems and data integrating models. The project was a multi-institutional collaboration with more than 20 active contributors. This presentation will describe the results of the water cycle component of the first phase of the project, which include seasonal (monthly) climatologies of water fluxes over land, ocean, and atmosphere at continental and ocean basin scales. The requirement of closure of the water budget (i.e., mass conservation) at various scales was exploited to constrain the flux estimates via an optimization approach that will also be described. Further, error assessments were included with the input datasets, and we examine these in relation to inferred uncertainty in the optimized flux estimates in order to gauge our current ability to close the water budget within an expected uncertainty range.

  7. SEOM's Sentinel-3/OLCI' project CAWA: advanced GRASP aerosol retrieval

    NASA Astrophysics Data System (ADS)

    Dubovik, Oleg; litvinov, Pavel; Huang, Xin; Aspetsberger, Michael; Fuertes, David; Brockmann, Carsten; Fischer, Jürgen; Bojkov, Bojan

    2016-04-01

    The CAWA "Advanced Clouds, Aerosols and WAter vapour products for Sentinel-3/OLCI" ESA-SEOM project aims on the development of advanced atmospheric retrieval algorithms for the Sentinel-3/OLCI mission, and is prepared using Envisat/MERIS and Aqua/MODIS datasets. This presentation discusses mainly CAWA aerosol product developments and results. CAWA aerosol retrieval uses recently developed GRASP algorithm (Generalized Retrieval of Aerosol and Surface Properties) algorithm described by Dubovik et al. (2014). GRASP derives extended set of atmospheric parameters using multi-pixel concept - a simultaneous fitting of a large group of pixels under additional a priori constraints limiting the time variability of surface properties and spatial variability of aerosol properties. Over land GRASP simultaneously retrieves properties of both aerosol and underlying surface even over bright surfaces. GRAPS doesn't use traditional look-up-tables and performs retrieval as search in continuous space of solution. All radiative transfer calculations are performed as part of the retrieval. The results of comprehensive sensitivity tests, as well as results obtained from real Envisat/MERIS data will be presented. The tests analyze various aspects of aerosol and surface reflectance retrieval accuracy. In addition, the possibilities of retrieval improvement by means of implementing synergetic inversion of a combination of OLCI data with observations by SLSTR are explored. Both the results of numerical tests, as well as the results of processing several years of Envisat/MERIS data illustrate demonstrate reliable retrieval of AOD (Aerosol Optical Depth) and surface BRDF. Observed retrieval issues and advancements will be discussed. For example, for some situations we illustrate possibilities of retrieving aerosol absorption - property that hardly accessible from satellite observations with no multi-angular and polarimetric capabilities.

  8. Global Aerosol Optical Models and Lookup Tables for the New MODIS Aerosol Retrieval over Land

    NASA Technical Reports Server (NTRS)

    Levy, Robert C.; Remer, Loraine A.; Dubovik, Oleg

    2007-01-01

    Since 2000, MODIS has been deriving aerosol properties over land from MODIS observed spectral reflectance, by matching the observed reflectance with that simulated for selected aerosol optical models, aerosol loadings, wavelengths and geometrical conditions (that are contained in a lookup table or 'LUT'). Validation exercises have showed that MODIS tends to under-predict aerosol optical depth (tau) in cases of large tau (tau greater than 1.0), signaling errors in the assumed aerosol optical properties. Using the climatology of almucantur retrievals from the hundreds of global AERONET sunphotometer sites, we found that three spherical-derived models (describing fine-sized dominated aerosol), and one spheroid-derived model (describing coarse-sized dominated aerosol, presumably dust) generally described the range of observed global aerosol properties. The fine dominated models were separated mainly by their single scattering albedo (omega(sub 0)), ranging from non-absorbing aerosol (omega(sub 0) approx. 0.95) in developed urban/industrial regions, to neutrally absorbing aerosol (omega(sub 0) approx.90) in forest fire burning and developing industrial regions, to absorbing aerosol (omega(sub 0) approx. 0.85) in regions of savanna/grassland burning. We determined the dominant model type in each region and season, to create a 1 deg. x 1 deg. grid of assumed aerosol type. We used vector radiative transfer code to create a new LUT, simulating the four aerosol models, in four MODIS channels. Independent AERONET observations of spectral tau agree with the new models, indicating that the new models are suitable for use by the MODIS aerosol retrieval.

  9. Maritime Aerosol Network as a Component of AERONET - a Useful Tool for Evaluation of the Global Sea-Salt Aerosol Distribution

    NASA Astrophysics Data System (ADS)

    Smirnov, A.; Holben, B. N.; Kinne, S.; Nelson, N. B.; Stenchikov, G. L.; Broccardo, S. P.; Sowers, D.; Lobecker, E.; Ondrusek, M.; Zielinski, T. P.; Gray, L. M.; Frouin, R.; Radionov, V. F.; Smyth, T. J.; Zibordi, G.; Heller, M. I.; Slabakova, V.; Krüger, K.; Reid, E. A.; Istomina, L.; Vandermeulen, R. A.; O'Neill, N. T.; Levy, G.; Giles, D. M.; Slutsker, I.; Sorokin, M. G.; Eck, T. F.

    2016-02-01

    Sea-salt aerosol plays an important role in radiation balance and chemistry of marine atmosphere. Sea-salt production depends on various factors. There is a significant uncertainty in the parametrization of the sea-salt production and budget. Ship-based aerosol optical depth (AOD) measurements can be used as an important validation tool for various global models and in-situ measurements. The paper presents the current status of the Maritime Aerosol Network (MAN) which is a component of Aerosol Robotic Network. Since 2006 over 300 cruises were completed and data archive of more than 5500 measurement days is accessible at http://aeronet.gsfc.nasa.gov/new_web/maritime_aerosol_network.html . AOD measurements from ships of opportunity complemented island-based AERONET measurements and provided important reference points for satellite retrieved and modelled AOD climatology over the oceans. The program exemplifies mutually beneficial international, multi-agency effort in atmospheric aerosol optical studies over the oceans.

  10. Aerosol characteristics in north-east India using ARFINET spectral optical depth measurements

    NASA Astrophysics Data System (ADS)

    Pathak, B.; Subba, T.; Dahutia, P.; Bhuyan, P. K.; Moorthy, K. Krishna; Gogoi, M. M.; Babu, S. Suresh; Chutia, L.; Ajay, P.; Biswas, J.; Bharali, C.; Borgohain, A.; Dhar, P.; Guha, A.; De, B. K.; Banik, T.; Chakraborty, M.; Kundu, S. S.; Sudhakar, S.; Singh, S. B.

    2016-01-01

    Four years (2010-2014) of spectral aerosol optical depth (AOD) data from 4 Indian Space Research Organisation's ARFINET (Aerosol Radiative Forcing over India) stations (Shillong, Agartala, Imphal and Dibrugarh) in the North-Eastern Region (NER) of India (lying between 22-30°N and 89-98°E) are synthesized to evolve a regional aerosol representation, for the first time. Results show that the columnar AOD (an indicator of the column abundance of aerosols) is highest at Agartala (0.80 ± 0.24) in the west and lowest at Imphal (0.59 ± 0.23) in the east in the pre-monsoon season due to intense anthropogenic bio-mass burning in this region aided by long-range transport from the high aerosol laden regions of the Indo-Gangetic Plains (IGP), polluted Bangladesh and Bay of Bengal. In addition to local biogenic aerosols and pollutants emitted from brick kilns, oil/gas fields, household bio-fuel/fossil-fuel, vehicles, industries. Aerosol distribution and climatic impacts show a west to east gradient within the NER. For example, the climatological mean AODs are 0.67 ± 0.26, 0.52 ± 0.14, 0.40 ± 0.17 and 0.41 ± 0.23 respectively in Agartala, Shillong, Imphal and Dibrugarh which are geographically located from west to east within the NER. The average aerosol burden in NER ranks second highest with climatological mean AOD 0.49 ± 0.2 next to the Indo-Gangetic Plains where the climatological mean AOD is 0.64 ± 0.2 followed by the South and South-East Asia region. Elevated aerosol layers are observed over the eastern most stations Dibrugarh and Imphal, while at the western stations the concentrations are high near the surface. The climate implications of aerosols are evaluated in terms of aerosol radiative forcing (ARF) and consequent heating of the atmosphere in the region which follows AOD and exhibit high values in pre-monsoon season at all the locations except in Agartala. The highest ARF in the atmosphere occurs in the pre-monsoon season ranging from 48.6 Wm-2 in Agartala

  11. NEWS Climatology Project: The State of the Water Cycle at Continental to Global Scales

    NASA Technical Reports Server (NTRS)

    Rodell, Matthew; LEcuyer, Tristan; Beaudoing, Hiroko Kato; Olson, Bill

    2011-01-01

    NASA's Energy and Water Cycle Study (NEWS) program fosters collaborative research towards improved quantification and prediction of water and energy cycle consequences of climate change. In order to measure change, it is first necessary to describe current conditions. The goal of the NEWS Water and Energy Cycle Climatology project is to develop "state of the global water cycle" and "state of the global energy cycle" assessments based on data from modern ground and space based observing systems and data integrating models. The project is a multiinstitutional collaboration with more than 20 active contributors. This presentation will describe results of the first stage of the water budget analysis, whose goal was to characterize the current state of the water cycle on mean monthly, continental scales. We examine our success in closing the water budget within the expected uncertainty range and the effects of forcing budget closure as a method for refining individual flux estimates.

  12. The New 20-Year Global Precipitation Climatology Project (GPCP) Merged Satellite and Rainguage Monthly Analysis

    NASA Technical Reports Server (NTRS)

    Adler, Robert; Huffman, George; Xie, Ping Ping; Rudolf, Bruno; Gruber, Arnold; Janowiak, John

    1999-01-01

    A new 20-year, monthly, globally complete precipitation analysis has been completed as part of the World Climate Research Program's (WCRP/GEWEX) Global Precipitation Climatology Project (GPCP). This Version 2 of the community generated data set is a result of combining the procedures and data sets as described. The global, monthly, 2.5x 2.5 degree latitude-longitude product utilizes precipitation estimates from low-orbit microwave sensors (SSM/1) and geosynchronous IR sensors and raingauge information over land. The low-orbit microwave estimates are used to adjust or correct the geosynchronous IR estimates, thereby maximizing the utility of the more physically-based microwave estimates and the finer time sampling of the geosynchronous observations. Information from raingauges is blended into the analyses over land. In the 1986-present period TOVS-based precipitation estimates are adjusted to GPCP fields and used in polar regions to produce globally-complete results. The extension back to 1979 utilizes the procedures of Xie and Arkin and their OLR Precipitation Index (OPI). The 20-year climatology of the Version 2 GPCP analysis indicates the expected features of a very strong Pacific Ocean ITCZ and SPCZ with maximum 20-year means approaching 10 mm/day. A similar strength maximum over land is evident over Borneo. Weaker maxima in the tropics occur in the Atlantic ITCZ and over South America and Africa. In mid-latitudes of the Northern Hemisphere the Western Pacific and Western Atlantic maxima have values of approximately 7 mm/day, while in the Southern Hemisphere the mid-latitude maxima are located southeast of Africa, in mid-Pacific as an extension of the SPCZ and southeast of South America. In terms of global totals the GPCP analysis shows 2.7 mm/day (3.0 mm/day over ocean; 2.1 mm/day over land), similar to the Jaeger climatology, but not other climatologies. Zonal averages peak at 6 mm/day at 7*N with mid-latitude peaks of about 3 mm/day at 40-45* latitude

  13. Aerosol optical properties over the midcontinental United States

    NASA Technical Reports Server (NTRS)

    Halthore, Rangasayi N.; Markham, Brian L.; Ferrare, Richard A.; Aro, Theo. O.

    1992-01-01

    Solar and sky radiation measurements were analyzed to obtain aerosol properties such as the optical thickness and the size distribution. The measurements were conducted as part of the First International Satellite Land Surface Climatology Project Field Experiment during the second intensive field campaign (IFC) from June 25 to July 14, 1987, and the fifth IFC from July 25 to August 12, 1989, on the Konza Prairie near Manhattan, Kansas. Correlations with climatological and meteorological parameters show that during the period of observations in 1987, two types of air masses dominated the area: an air mass with low optical thickness and low temperature air associated with a northerly breeze, commonly referred to as the continental air, and an air mass with a higher optical thickness and higher temperature air associated with a southerly wind which we call 'Gulf air'. The size distributions show a predominance of the larger size particles in 'Gulf air'. Because of the presence of two contrasting air masses, correlations with parameters such as relative humidity, specific humidity, pressure, temperature, and North Star sky radiance reveal some interesting aspects. In 1989, clear distinctions between continental and Gulf air cannot be made; the reason for this will be discussed.

  14. Impacts of increasing the aerosol complexity in the Met Office global NWP model

    NASA Astrophysics Data System (ADS)

    Mulcahy, Jane; Walters, David; Bellouin, Nicolas; Milton, Sean

    2014-05-01

    Inclusion of the direct and indirect radiative effects of aerosols in high resolution global numerical weather prediction (NWP) models is being increasingly recognised as important for the improved accuracy of short-range weather forecasts. In this study the impacts of increasing the aerosol complexity in the global NWP configuration of the Met Office Unified Model (MetUM) are investigated. A hierarchy of aerosol representations are evaluated including three dimensional monthly mean speciated aerosol climatologies, fully prognostic aerosols modelled using the CLASSIC aerosol scheme and finally, initialised aerosols using assimilated aerosol fields from the GEMS project. The prognostic aerosol schemes are better able to predict the temporal and spatial variation of atmospheric aerosol optical depth, which is particularly important in cases of large sporadic aerosol events such as large dust storms or forest fires. Including the direct effect of aerosols improves model biases in outgoing longwave radiation over West Africa due to a better representation of dust. Inclusion of the indirect aerosol effects has significant impacts on the SW radiation particularly at high latitudes due to lower cloud amounts in high latitude clean air regions. This leads to improved surface radiation biases at the North Slope of Alaska ARM site. Verification of temperature and height forecasts is also improved in this region. Impacts on the global mean model precipitation and large-scale circulation fields were found to be generally small in the short range forecasts. However, the indirect aerosol effect leads to a strengthening of the low level monsoon flow over the Arabian Sea and Bay of Bengal and an increase in precipitation over Southeast Asia. This study highlights the importance of including a more realistic treatment of aerosol-cloud interactions in global NWP models and the potential for improved global environmental prediction systems through the incorporation of more complex

  15. Model representations of aerosol layers transported from North America over the Atlantic Ocean during the Two-Column Aerosol Project

    NASA Astrophysics Data System (ADS)

    Fast, Jerome D.; Berg, Larry K.; Zhang, Kai; Easter, Richard C.; Ferrare, Richard A.; Hair, Johnathan W.; Hostetler, Chris A.; Liu, Ying; Ortega, Ivan; Sedlacek, Arthur; Shilling, John E.; Shrivastava, Manish; Springston, Stephen R.; Tomlinson, Jason M.; Volkamer, Rainer; Wilson, Jacqueline; Zaveri, Rahul A.; Zelenyuk, Alla

    2016-08-01

    The ability of the Weather Research and Forecasting model with chemistry (WRF-Chem) version 3.7 and the Community Atmosphere Model version 5.3 (CAM5) in simulating profiles of aerosol properties is quantified using extensive in situ and remote sensing measurements from the Two-Column Aerosol Project (TCAP) conducted during July of 2012. TCAP was supported by the U.S. Department of Energy's Atmospheric Radiation Measurement program and was designed to obtain observations within two atmospheric columns; one fixed over Cape Cod, Massachusetts, and the other several hundred kilometers over the ocean. The performance is quantified using most of the available aircraft and surface measurements during July, and 2 days are examined in more detail to identify the processes responsible for the observed aerosol layers. The higher-resolution WRF-Chem model produced more aerosol mass in the free troposphere than the coarser-resolution CAM5 model so that the fraction of aerosol optical thickness above the residual layer from WRF-Chem was more consistent with lidar measurements. We found that the free troposphere layers are likely due to mean vertical motions associated with synoptic-scale convergence that lifts aerosols from the boundary layer. The vertical displacement and the time period associated with upward transport in the troposphere depend on the strength of the synoptic system and whether relatively high boundary layer aerosol concentrations are present where convergence occurs. While a parameterization of subgrid scale convective clouds applied in WRF-Chem modulated the concentrations of aerosols aloft, it did not significantly change the overall altitude and depth of the layers.

  16. Reallocation in modal aerosol models: impacts on predicting aerosol radiative effects

    NASA Astrophysics Data System (ADS)

    Korhola, T.; Kokkola, H.; Korhonen, H.; Partanen, A.-I.; Laaksonen, A.; Lehtinen, K. E. J.; Romakkaniemi, S.

    2013-08-01

    In atmospheric modelling applications the aerosol particle size distribution is commonly represented by modal approach, in which particles in different size ranges are described with log-normal modes within predetermined size ranges. Such method includes numerical reallocation of particles from a mode to another for example during particle growth, leading to potentially artificial changes in the aerosol size distribution. In this study we analysed how this reallocation affects climatologically relevant parameters: cloud droplet number concentration, aerosol-cloud interaction coefficient and light extinction coefficient. We compared these parameters between a modal model with and without reallocation routines, and a high resolution sectional model that was considered as a reference model. We analysed the relative differences of the parameters in different experiments that were designed to cover a wide range of dynamic aerosol processes occurring in the atmosphere. According to our results, limiting the allowed size ranges of the modes and the following numerical remapping of the distribution by reallocation, leads on average to underestimation of cloud droplet number concentration (up to 100%) and overestimation of light extinction (up to 20%). The analysis of aerosol first indirect effect is more complicated as the ACI parameter can be either over- or underestimated by the reallocating model, depending on the conditions. However, for example in the case of atmospheric new particle formation events followed by rapid particle growth, the reallocation can cause around average 10% overestimation of the ACI parameter. Thus it is shown that the reallocation affects the ability of a model to estimate aerosol climate effects accurately, and this should be taken into account when using and developing aerosol models.

  17. Status and Plans for the WCRP/GEWEX Global Precipitation Climatology Project (GPCP)

    NASA Technical Reports Server (NTRS)

    Adler, Robert F.

    2007-01-01

    The Global Precipitation Climatology Project (GPCP) is an international project under the auspices of the World Climate Research Program (WCRP) and GEWEX (Global Water and Energy Experiment). The GPCP group consists of scientists from agencies and universities in various countries that work together to produce a set of global precipitation analyses at time scales of monthly, pentad, and daily. The status of the current products will be briefly summarized, focusing on the monthly analysis. Global and large regional rainfall variations and possible long-term changes are examined using the 27-year (1 979-2005) monthly dataset. In addition to global patterns associated with phenomena such as ENSO, the data set is explored for evidence of long-term change. Although the global change of precipitation in the data set is near zero, the data set does indicate a small upward change in the Tropics (25s-25N) during the period,. especially over ocean. Techniques are derived to isolate and eliminate variations due to ENS0 and major volcanic eruptions and the significance of the linear change is examined. Plans for a GPCP reprocessing for a Version 3 of products, potentially including a fine-time resolution product will be discussed. Current and future links to IPWG will also be addressed.

  18. Smart Climatology Applications for Undersea Warfare

    DTIC Science & Technology

    2008-09-01

    Comparisons of these climatologies with existing Navy climatologies based on the Generalized Digital Environmental Model ( GDEM ) reveal differences in sonic...undersea warfare. 15. NUMBER OF PAGES 117 14. SUBJECT TERMS antisubmarine warfare, climate variations, climatology, GDEM , ocean, re...climatologies based on the Generalized Digital Environmental Model ( GDEM ) to our smart ocean climatologies reveal a number of differences. The

  19. SeReNA Project: studying aerosol interactions with cloud microphysics in the Amazon Basin

    NASA Astrophysics Data System (ADS)

    Correia, A. L.; Catandi, P. B.; Frigeri, F. F.; Ferreira, W. C.; Martins, J.; Artaxo, P.

    2012-12-01

    Cloud microphysics and its interaction with aerosols is a key atmospheric process for weather and climate. Interactions between clouds and aerosols can impact Earth's radiative balance, its hydrological and energetic cycles, and are responsible for a large fraction of the uncertainty in climatic models. On a planetary scale, the Amazon Basin is one of the most significant land sources of moisture and latent heat energy. Moreover, every year this region undergoes mearked seasonal shifts in its atmospheric state, transitioning from clean to heavily polluted conditions due to the occurrence of seasonal biomass burning fires, that emit large amounts of smoke to the atmosphere. These conditions make the Amazon Basin a special place to study aerosol-cloud interactions. The SeReNA Project ("Remote sensing of clouds and their interaction with aerosols", from the acronym in Portuguese, @SerenaProject on Twitter) is an ongoing effort to experimentally investigate the impact of aerosols upon cloud microphysics in Amazonia. Vertical profiles of droplet effective radius of water and ice particles, in single convective clouds, can be derived from measurements of the emerging radiation on cloud sides. Aerosol optical depth, cloud top properties, and meteorological parameters retrieved from satellites will be correlated with microphysical properties derived for single clouds. Maps of cloud brightness temperature will allow building temperature vs. effective radius profiles for hydrometeors in single clouds. Figure 1 shows an example extracted from Martins et al. (2011), illustrating a proof-of-concept for the kind of result expected within the framework for the SeReNA Project. The results to be obtained will help foster the quantitative knowledge about interactions between aerosols and clouds in a microphysical level. These interactions are a fundamental process in the context of global climatic changes, they are key to understanding basic processes within clouds and how aerosols

  20. Model representations of aerosol layers transported from North America over the Atlantic Ocean during the Two-Column Aerosol Project

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Fast, Jerome D.; Berg, Larry K.; Zhang, Kai

    2016-08-22

    The ability of the Weather Research and Forecasting model with chemistry (WRF-Chem) version 3.7 and the Community Atmosphere Model version 5.3 (CAM5) in simulating profiles of aerosol properties is quantified using extensive in situ and remote sensing measurements from the Two Column Aerosol Project (TCAP) conducted during July of 2012. TCAP was supported by the U.S. Department of Energy’s Atmospheric Radiation Measurement program and was designed to obtain observations within two atmospheric columns; one fixed over Cape Cod, Massachusetts and the other several hundred kilometers over the ocean. The performance is quantified using most of the available aircraft and surfacemore » measurements during July, and two days are examined in more detail to identify the processes responsible for the observed aerosol layers. The higher resolution WRF-Chem model produced more aerosol mass in the free troposphere than the coarser resolution CAM5 model so that the fraction of aerosol optical thickness above the residual layer from WRF-Chem was more consistent with lidar measurements. We found that the free troposphere layers are likely due to mean vertical motions associated with synoptic-scale convergence that lifts aerosols from the boundary layer. The vertical displacement and the time period associated with upward transport in the troposphere depend on the strength of the synoptic system and whether relatively high boundary layer aerosol concentrations are present where convergence occurs. While a parameterization of subgrid scale convective clouds applied in WRF-Chem modulated the concentrations of aerosols aloft, it did not significantly change the overall altitude and depth of the layers.« less

  1. Model representations of aerosol layers transported from North America over the Atlantic Ocean during the Two-Column Aerosol Project

    DOE PAGES

    Fast, Jerome D.; Berg, Larry K.; Zhang, Kai; ...

    2016-08-22

    The ability of the Weather Research and Forecasting model with chemistry (WRF-Chem) version 3.7 and the Community Atmosphere Model version 5.3 (CAM5) in simulating profiles of aerosol properties is quantified using extensive in situ and remote sensing measurements from the Two-Column Aerosol Project (TCAP) conducted during July of 2012. TCAP was supported by the U.S. Department of Energy's Atmospheric Radiation Measurement program and was designed to obtain observations within two atmospheric columns; one fixed over Cape Cod, Massachusetts, and the other several hundred kilometers over the ocean. The performance is quantified using most of the available aircraft and surface measurementsmore » during July, and 2 days are examined in more detail to identify the processes responsible for the observed aerosol layers. The higher-resolution WRF-Chem model produced more aerosol mass in the free troposphere than the coarser-resolution CAM5 model so that the fraction of aerosol optical thickness above the residual layer from WRF-Chem was more consistent with lidar measurements. We found that the free troposphere layers are likely due to mean vertical motions associated with synoptic-scale convergence that lifts aerosols from the boundary layer. The vertical displacement and the time period associated with upward transport in the troposphere depend on the strength of the synoptic system and whether relatively high boundary layer aerosol concentrations are present where convergence occurs. In conclusion, while a parameterization of subgrid scale convective clouds applied in WRF-Chem modulated the concentrations of aerosols aloft, it did not significantly change the overall altitude and depth of the layers.« less

  2. The OMI Aerosol Absorption Product: An A-train application

    NASA Astrophysics Data System (ADS)

    Torres, O.; Jethva, H. T.; Ahn, C.

    2017-12-01

    Because of the uniquely large sensitivity of satellite-measured near-UV radiances to absorption by desert dust, carbonaceous and volcanic ash aerosols, observations by a variety of UV-capable sensors have been routinely used over the last forty years in both qualitative and quantitative applications for estimating the absorption properties of these aerosol types. In this presentation we will discuss a multi-sensor application involving observations from A-train sensors OMI, AIRS and CALIOP for the creation of a 13-year record of aerosol optical depth (AOD) and single scattering albedo (SSA). Determination of aerosol type, in terms of particle size distribution and refractive index, is an important algorithmic step that requires using external information. AIRS CO measurements are used as carbonaceous aerosols tracer to differentiate this aerosol type from desert dust. On the other hand, the height of the absorbing aerosol layer, an important parameter in UV aerosol retrievals, is prescribed using a CALIOP-based climatology. The combined use of these observations in the developments of the OMI long-term AOD/SSA record will be discussed along with an evaluation of retrieval results using independent observations.

  3. Trends in Ocean Irradiance using a Radiative Model Forced with Terra Aerosols and Clouds

    NASA Technical Reports Server (NTRS)

    Gregg, Watson; Casey, Nancy; Romanou, Anastasia

    2010-01-01

    Aerosol and cloud information from MODIS on Terra provide enhanced capability to understand surface irradiance over the oceans and its variability. These relationships can be important for ocean biology and carbon cycles. An established radiative transfer model, the Ocean-Atmosphere Spectral Irradiance Model (OASIM) is used to describe ocean irradiance variability on seasonal to decadal time scales. The model is forced with information on aerosols and clouds from the MODIS sensor on Terra and Aqua. A 7-year record (2000-2006) showed no trends in global ocean surface irradiance or photosynthetic available irradiance (PAR). There were significant (P<0.05) negative trends in the Mediterranean Sea, tropical Pacific) and tropical Indian Oceans, of -7.0, -5.0 and -2.7 W/sq m respectively. Global interannual variability was also modest. Regional interannual variability was quite large in some ocean basins, where monthly excursions from climatology were often >20 W/sq m. The trends using MODIS data contrast with results from OASIM using liquid water path estimates from the International Satellite Cloud Climatology Project (ISCCP). Here, a global trend of -2 W/sq m was observed, largely dues to a large negative trend in the Antarctic -12 W/sq m. These results suggest the importance of the choice of liquid water path data sets in assessments of medium-length trends in ocean surface irradiance. The choices also impact the evaluation of changes in ocean biogeochemistry.

  4. A Global Data Assimilation System for Atmospheric Aerosol

    NASA Technical Reports Server (NTRS)

    daSilva, Arlindo

    1999-01-01

    We will give an overview of an aerosol data assimilation system which combines advances in remote sensing of atmospheric aerosols, aerosol modeling and data assimilation methodology to produce high spatial and temporal resolution 3D aerosol fields. Initially, the Goddard Aerosol Assimilation System (GAAS) will assimilate TOMS, AVHRR and AERONET observations; later we will include MODIS and MISR. This data assimilation capability will allows us to integrate complementing aerosol observations from these platforms, enabling the development of an assimilated aerosol climatology as well as a global aerosol forecasting system in support of field campaigns. Furthermore, this system provides an interactive retrieval framework for each aerosol observing satellites, in particular TOMS and AVHRR. The Goddard Aerosol Assimilation System (GAAS) takes advantage of recent advances in constituent data assimilation at DAO, including flow dependent parameterizations of error covariances and the proper consideration of model bias. For its prognostic transport model, GAAS will utilize the Goddard Ozone, Chemistry, Aerosol, Radiation and Transport (GOCART) model developed at NASA/GSFC Codes 916 and 910.3. GOCART includes the Lin-Rood flux-form, semi-Langrangian transport model with parameterized aerosol chemistry and physical processes for absorbing (dust and black carbon) and non-absorbing aerosols (sulfate and organic carbon). Observations and model fields are combined using a constituent version of DAO's Physical-space Statistical Analysis System (PSAS), including its adaptive quality control system. In this talk we describe the main components of this assimilation system and present preliminary results obtained by assimilating TOMS data.

  5. A new approach to correct for absorbing aerosols in OMI UV

    NASA Astrophysics Data System (ADS)

    Arola, A.; Kazadzis, S.; Lindfors, A.; Krotkov, N.; Kujanpää, J.; Tamminen, J.; Bais, A.; di Sarra, A.; Villaplana, J. M.; Brogniez, C.; Siani, A. M.; Janouch, M.; Weihs, P.; Webb, A.; Koskela, T.; Kouremeti, N.; Meloni, D.; Buchard, V.; Auriol, F.; Ialongo, I.; Staneck, M.; Simic, S.; Smedley, A.; Kinne, S.

    2009-11-01

    Several validation studies of surface UV irradiance based on the Ozone Monitoring Instrument (OMI) satellite data have shown a high correlation with ground-based measurements but a positive bias in many locations. The main part of the bias can be attributed to the boundary layer aerosol absorption that is not accounted for in the current satellite UV algorithms. To correct for this shortfall, a post-correction procedure was applied, based on global climatological fields of aerosol absorption optical depth. These fields were obtained by using global aerosol optical depth and aerosol single scattering albedo data assembled by combining global aerosol model data and ground-based aerosol measurements from AERONET. The resulting improvements in the satellite-based surface UV irradiance were evaluated by comparing satellite and ground-based spectral irradiances at various European UV monitoring sites. The results generally showed a significantly reduced bias by 5-20%, a lower variability, and an unchanged, high correlation coefficient.

  6. Aerosol Optical Depth Distribution in Extratropical Cyclones over the Northern Hemisphere Oceans

    NASA Technical Reports Server (NTRS)

    Naud, Catherine M.; Posselt, Derek J.; van den Heever, Susan C.

    2016-01-01

    Using Moderate Resolution Imaging Spectroradiometer and an extratropical cyclone database,the climatological distribution of aerosol optical depth (AOD) in extratropical cyclones is explored based solely on observations. Cyclone-centered composites of aerosol optical depth are constructed for the Northern Hemisphere mid-latitude ocean regions, and their seasonal variations are examined. These composites are found to be qualitatively stable when the impact of clouds and surface insolation or brightness is tested. The larger AODs occur in spring and summer and are preferentially found in the warm frontal and in the post-cold frontal regions in all seasons. The fine mode aerosols dominate the cold sector AODs, but the coarse mode aerosols display large AODs in the warm sector. These differences between the aerosol modes are related to the varying source regions of the aerosols and could potentially have different impacts on cloud and precipitation within the cyclones.

  7. A Global Ozone Climatology from Ozone Soundings via Trajectory Mapping: A Stratospheric Perspective

    NASA Technical Reports Server (NTRS)

    Liu, J. J.; Tarasick, D. W.; Fioletov, V. E.; McLinden, C.; Zhao, T.; Gong, S.; Sioris, G.; Jin, J. J.; Liu, G.; Moeini, O.

    2013-01-01

    This study explores a domain-filling trajectory approach to generate a global ozone climatology from sparse ozonesonde data. Global ozone soundings of 51,898 profiles at 116 stations over 44 years (1965-2008) are used, from which forward and backward trajectories are performed for 4 days, driven by a set of meteorological reanalysis data. Ozone mixing ratios of each sounding from the surface to 26 km altitude are assigned to the entire path along the trajectory. The resulting global ozone climatology is archived monthly for five decades from the 1960s to the 2000s with grids of 5 degree 5 degree 1 km (latitude, longitude, and altitude). It is also archived yearly from 1965 to 2008. This climatology is validated at 20 ozonesonde stations by comparing the actual ozone sounding profile with that found through the trajectories, using the ozone soundings at all the stations except one being tested. The two sets of profiles are in good agreement, both individually with correlation coefficients between 0.975 and 0.998 and root mean square (RMS) differences of 87 to 482 ppbv, and overall with a correlation coefficient of 0.991 and an RMS of 224 ppbv. The ozone climatology is also compared with two sets of satellite data, from the Satellite Aerosol and Gas Experiment (SAGE) and the Optical Spectrography and InfraRed Imager System (OSIRIS). Overall, the ozone climatology compares well with SAGE and OSIRIS data by both seasonal and zonal means. The mean difference is generally under 20 above 15 km. The comparison is better in the northern hemisphere, where there are more ozonesonde stations, than in the southern hemisphere; it is also better in the middle and high latitudes than in the tropics, where assimilated winds are imperfect in some regions. This ozone climatology can capture known features in the stratosphere, as well as seasonal and decadal variations of these features. Furthermore, it provides a wealth of detail about longitudinal variations in the stratosphere such

  8. Two-Channel Satellite Retrievals of Aerosol Properties: An Overview

    NASA Technical Reports Server (NTRS)

    Mishchenko, Michael I.

    1999-01-01

    In order to reduce current uncertainties in the evaluation of the direct and indirect effects of tropospheric aerosols on climate on the global scale, it has been suggested to apply multi-channel retrieval algorithms to the full period of existing satellite data. This talk will outline the methodology of interpreting two-channel satellite radiance data over the ocean and describe a detailed analysis of the sensitivity of retrieved aerosol parameters to the assumptions made in different retrieval algorithms. We will specifically address the calibration and cloud screening issues, consider the suitability of existing satellite data sets to detecting short- and long-term regional and global changes, compare preliminary results obtained by several research groups, and discuss the prospects of creating an advanced retroactive climatology of aerosol optical thickness and size over the oceans.

  9. An updated climatology of surface dimethlysulfide concentrations and emission fluxes in the global ocean

    NASA Astrophysics Data System (ADS)

    Lana, A.; Bell, T. G.; Simó, R.; Vallina, S. M.; Ballabrera-Poy, J.; Kettle, A. J.; Dachs, J.; Bopp, L.; Saltzman, E. S.; Stefels, J.; Johnson, J. E.; Liss, P. S.

    2011-03-01

    The potentially significant role of the biogenic trace gas dimethylsulfide (DMS) in determining the Earth's radiation budget makes it necessary to accurately reproduce seawater DMS distribution and quantify its global flux across the sea/air interface. Following a threefold increase of data (from 15,000 to over 47,000) in the global surface ocean DMS database over the last decade, new global monthly climatologies of surface ocean DMS concentration and sea-to-air emission flux are presented as updates of those constructed 10 years ago. Interpolation/extrapolation techniques were applied to project the discrete concentration data onto a first guess field based on Longhurst's biogeographic provinces. Further objective analysis allowed us to obtain the final monthly maps. The new climatology projects DMS concentrations typically in the range of 1-7 nM, with higher levels occurring in the high latitudes, and with a general trend toward increasing concentration in summer. The increased size and distribution of the observations in the DMS database have produced in the new climatology substantially lower DMS concentrations in the polar latitudes and generally higher DMS concentrations in regions that were severely undersampled 10 years ago, such as the southern Indian Ocean. Using the new DMS concentration climatology in conjunction with state-of-the-art parameterizations for the sea/air gas transfer velocity and climatological wind fields, we estimate that 28.1 (17.6-34.4) Tg of sulfur are transferred from the oceans into the atmosphere annually in the form of DMS. This represents a global emission increase of 17% with respect to the equivalent calculation using the previous climatology. This new DMS climatology represents a valuable tool for atmospheric chemistry, climate, and Earth System models.

  10. Aerosol-driven increase in Arctic sea ice over the middle of the twentieth century

    NASA Astrophysics Data System (ADS)

    Gagné, Marie-Ève; Fyfe, John C.; Gillett, Nathan P.; Polyakov, Igor V.; Flato, Gregory M.

    2017-07-01

    Updated observational data sets without climatological infilling show that there was an increase in sea ice concentration in the eastern Arctic between 1950 and 1975, contrary to earlier climatology infilled observational data sets that show weak interannual variations during that time period. We here present climate model simulations showing that this observed sea ice concentration increase was primarily a consequence of cooling induced by increasing anthropogenic aerosols and natural forcing. Indeed, sulphur dioxide emissions, which lead to the formation of sulphate aerosols, peaked around 1980 causing a sharp increase in the burden of sulphate between the 1950s and 1970s; but since 1980, the burden has dropped. Our climate model simulations show that the cooling contribution of aerosols offset the warming effect of increasing greenhouse gases over the midtwentieth century resulting in the expansion of the Arctic sea ice cover. These results challenge the perception that Arctic sea ice extent was unperturbed by human influence until the 1970s, suggesting instead that it exhibited earlier forced multidecadal variations, with implications for our understanding of impacts and adaptation in human and natural Arctic systems.

  11. The Remote Sensing of Mineral Aerosols and their Impact on Phytoplankton Productivity

    NASA Technical Reports Server (NTRS)

    Tindale, Neil W.

    1997-01-01

    The overall objective of this experiment was to test the iron hypothesis does the addition of iron to nutrient rich surface waters enhance productivity? Our specific objectives in this experiment included sampling and studying the marine aerosol size and type (which are related to chemical reactivity) during the PlumEx cruise to determine the importance of local (Galapagos Islands) versus long-range sources of atmospheric material. Detailed results of single particle analysis of our samples are being prepared for publication in two papers. We collect aerosol samples and they have been analyzed for trace metals and other elements. We are mapped aerosol distribution and the desert source areas around the Arabian Sea region. We did record a clear relationship between the aerosol radiance and synoptic weather patterns with distinct signals over the ocean northwest and southwest of Australia. While the interpretation was limited an aerosol climatology pattern was presented.

  12. Stratospheric Aerosol--Observations, Processes, and Impact on Climate

    NASA Technical Reports Server (NTRS)

    Kresmer, Stefanie; Thomason, Larry W.; von Hobe, Marc; Hermann, Markus; Deshler, Terry; Timmreck, Claudia; Toohey, Matthew; Stenke, Andrea; Schwarz, Joshua P.; Weigel, Ralf; hide

    2016-01-01

    Interest in stratospheric aerosol and its role in climate have increased over the last decade due to the observed increase in stratospheric aerosol since 2000 and the potential for changes in the sulfur cycle induced by climate change. This review provides an overview about the advances in stratospheric aerosol research since the last comprehensive assessment of stratospheric aerosol was published in 2006. A crucial development since 2006 is the substantial improvement in the agreement between in situ and space-based inferences of stratospheric aerosol properties during volcanically quiescent periods. Furthermore, new measurement systems and techniques, both in situ and space based, have been developed for measuring physical aerosol properties with greater accuracy and for characterizing aerosol composition. However, these changes induce challenges to constructing a long-term stratospheric aerosol climatology. Currently, changes in stratospheric aerosol levels less than 20% cannot be confidently quantified. The volcanic signals tend to mask any nonvolcanically driven change, making them difficult to understand. While the role of carbonyl sulfide as a substantial and relatively constant source of stratospheric sulfur has been confirmed by new observations and model simulations, large uncertainties remain with respect to the contribution from anthropogenic sulfur dioxide emissions. New evidence has been provided that stratospheric aerosol can also contain small amounts of nonsulfatematter such as black carbon and organics. Chemistry-climate models have substantially increased in quantity and sophistication. In many models the implementation of stratospheric aerosol processes is coupled to radiation and/or stratospheric chemistry modules to account for relevant feedback processes.

  13. Answering the Call for Model-Relevant Observations of Aerosols and Clouds

    NASA Technical Reports Server (NTRS)

    Redemann, J.; Shinozuka, Y.; Kacenelenbogen, M.; Segal-Rozenhaimer, M.; LeBlanc, S.; Vaughan, M.; Stier, P.; Schutgens, N.

    2017-01-01

    We describe a technique for combining multiple A-Train aerosol data sets, namely MODIS spectral AOD (aerosol optical depth), OMI AAOD (absorption aerosol optical depth) and CALIOP aerosol backscatter retrievals (hereafter referred to as MOC retrievals) to estimate full spectral sets of aerosol radiative properties, and ultimately to calculate the 3-D distribution of direct aerosol radiative effects (DARE). We present MOC results using almost two years of data collected in 2007 and 2008, and show comparisons of the aerosol radiative property estimates to collocated AERONET retrievals. We compare the spatio-temporal distribution of the MOC retrievals and MOC-based calculations of seasonal clear-sky DARE to values derived from four models that participated in the Phase II AeroCom model intercomparison initiative. Comparisons of seasonal aerosol property to AeroCom Phase II results show generally good agreement best agreement with forcing results at TOA is found with GMI-MerraV3.We discuss the challenges in making observations that really address deficiencies in models, with some of the more relevant aspects being representativeness of the observations for climatological states, and whether a given model-measurement difference addresses a sampling or a model error.

  14. A comparison of the Stratospheric Aerosol and Gas Experiment II tropospheric water vapor to radiosonde measurements

    NASA Technical Reports Server (NTRS)

    Larsen, J. C.; Chiou, E. W.; Chu, W. P.; Mccormick, M. P.; Mcmaster, L. R.; Oltmans, S.; Rind, D.

    1993-01-01

    Results are presented of a comparison beteen observations of the upper-tropospheric water vapor data obtained from the Stratospheric Aerosol and Gas Experiment II (SAGE II) instrument and radiosonde observations for 1987 and radiosonde-based climatologies. Colocated SAGE II-radiosonde measurement pairs are compared individually and in a zonal mean sense. A straight comparison of monthly zonal means between SAGE II and radiosondes for 1987 and Global Atmospheric Statistics (1963-1973) indicates that the clear-sky SAGE II climatology is approximately half the level of clear/cloudy sky of both radiosonde climatologies. Annual zonal means calculated from the set of profile pairs again showed SAGE II to be significantly drier in many altitude bands.

  15. A global monthly sea surface temperature climatology

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Shea, D.J.; Trenberth, K.E.; Reynolds, R.W.

    1992-09-01

    The paper presents a new global 2 deg x 2 deg monthly sea surface temperature (SST) climatology, referred here to as the Shea-Trenberth-Reynolds (STR) climatology, which was derived by modifying a 1950-1979-based SST climatology from the Climate Analysis Center (CAC), by using data from the Comprehensive Ocean-Atmosphere Data Set to improve the SST estimates in the regions of the Kuroshio and the Gulf Stream. A comparison of the STR climatology with the Alexander and Mobley SST climatology showed that the STR climatology is warmer in the Northern Hemisphere, and colder poleward of 45 deg S. 22 refs.

  16. Aerosol Remote Sensing from Space - Where We Stand, Where We're Heading

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph

    2012-01-01

    The MISR and MODIS instruments aboard the NASA Earth Observing System's Terra Satellite have been collecting data containing information about the state of Earth's atmosphere and surface for over twelve years. Among the retrieved quantities are the amount and type of wildfire smoke, desert dust, volcanic effluent, urban and industrial pollution particles, and other aerosols. Data from these instruments have been used to develop a global, monthly climatology of aerosol amount that is widely used as a constraint on climate models, including those used for the 2007 IPCC assessment report. However, the broad scientific challenges of understanding aerosol impacts on climate and health place different, and very exacting demands on our measurement capabilities. And these data sets, though much more advanced in many respects than previous aerosol data records, are imperfect. The next frontier in assessing aerosol radiative forcing of climate is aerosol type, and in particular, the absorption properties of major aerosol air masses. In this presentation, I will summarize current understanding of MISR and MODIS aerosol product strengths and limitations, discuss how they relate to the bigger aerosol science questions we must address, and give my view of the way forward.

  17. The direct effect of aerosols on solar radiation over the broader Mediterranean basin

    NASA Astrophysics Data System (ADS)

    Papadimas, C. D.; Hatzianastassiou, N.; Matsoukas, C.; Kanakidou, M.; Mihalopoulos, N.; Vardavas, I.

    2012-08-01

    For the first time, the direct radiative effect (DRE) of aerosols on solar radiation is computed over the entire Mediterranean basin, one of the most climatically sensitive world regions, using a deterministic spectral radiation transfer model (RTM). The DRE effects on the outgoing shortwave radiation at the top of atmosphere (TOA), DRETOA, on the absorption of solar radiation in the atmospheric column, DREatm, and on the downward and absorbed surface solar radiation (SSR), DREsurf and DREnetsurf, respectively, are computed separately. The model uses input data for the period 2000-2007 for various surface and atmospheric parameters, taken from satellite (International Satellite Cloud Climatology Project, ISCCP-D2), Global Reanalysis projects (National Centers for Environmental Prediction - National Center for Atmospheric Research, NCEP/NCAR), and other global databases. The spectral aerosol optical properties (aerosol optical depth, AOD, asymmetry parameter, gaer and single scattering albedo, ωaer), are taken from the MODerate resolution Imaging Spectroradiometer (MODIS) of NASA (National Aeronautics and Space Administration) and they are supplemented by the Global Aerosol Data Set (GADS). The model SSR fluxes have been successfully validated against measurements from 80 surface stations of the Global Energy Balance Archive (GEBA) covering the period 2000-2007. A planetary cooling is found above the Mediterranean on an annual basis (regional mean DRETOA = -2.4 W m-2). Although a planetary cooling is found over most of the region, of up to -7 W m-2, large positive DRETOA values (up to +25 W m-2) are found over North Africa, indicating a strong planetary warming, and a weaker warming over the Alps (+0.5 W m-2). Aerosols are found to increase the absorption of solar radiation in the atmospheric column over the region (DREatm = +11.1 W m-2) and to decrease SSR (DREsurf = -16.5 W m-2 and DREnetsurf-13.5 W m-2) inducing thus significant atmospheric warming and surface

  18. Climatology 2011: An MLS and Sonde Derived Ozone Climatology for Satellite Retrieval Algorithms

    NASA Technical Reports Server (NTRS)

    McPeters, Richard D.; Labow, Gordon J.

    2012-01-01

    The ozone climatology used as the a priori for the version 8 Solar Backscatter Ultraviolet (SBUV) retrieval algorithms has been updated. The Microwave Limb Sounder (MLS) instrument on Aura has excellent latitude coverage and measures ozone daily from the upper troposphere to the lower mesosphere. The new climatology consists of monthly average ozone profiles for ten degree latitude zones covering pressure altitudes from 0 to 65 km. The climatology was formed by combining data from Aura MLS (2004-2010) with data from balloon sondes (1988-2010). Ozone below 8 km (below 12 km at high latitudes) is based on balloons sondes, while ozone above 16 km (21 km at high latitudes) is based on MLS measurements. Sonde and MLS data are blended in the transition region. Ozone accuracy in the upper troposphere is greatly improved because of the near uniform coverage by Aura MLS, while the addition of a large number of balloon sonde measurements improves the accuracy in the lower troposphere, in the tropics and southern hemisphere in particular. The addition of MLS data also improves the accuracy of climatology in the upper stratosphere and lower mesosphere. The revised climatology has been used for the latest reprocessing of SBUV and TOMS satellite ozone data.

  19. Minimum aerosol layer detection sensitivities and their subsequent impacts on aerosol optical thickness retrievals in CALIPSO level 2 data products

    NASA Astrophysics Data System (ADS)

    Toth, Travis D.; Campbell, James R.; Reid, Jeffrey S.; Tackett, Jason L.; Vaughan, Mark A.; Zhang, Jianglong; Marquis, Jared W.

    2018-01-01

    Due to instrument sensitivities and algorithm detection limits, level 2 (L2) Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) 532 nm aerosol extinction profile retrievals are often populated with retrieval fill values (RFVs), which indicate the absence of detectable levels of aerosol within the profile. In this study, using 4 years (2007-2008 and 2010-2011) of CALIOP version 3 L2 aerosol data, the occurrence frequency of daytime CALIOP profiles containing all RFVs (all-RFV profiles) is studied. In the CALIOP data products, the aerosol optical thickness (AOT) of any all-RFV profile is reported as being zero, which may introduce a bias in CALIOP-based AOT climatologies. For this study, we derive revised estimates of AOT for all-RFV profiles using collocated Moderate Resolution Imaging Spectroradiometer (MODIS) Dark Target (DT) and, where available, AErosol RObotic NEtwork (AERONET) data. Globally, all-RFV profiles comprise roughly 71 % of all daytime CALIOP L2 aerosol profiles (i.e., including completely attenuated profiles), accounting for nearly half (45 %) of all daytime cloud-free L2 aerosol profiles. The mean collocated MODIS DT (AERONET) 550 nm AOT is found to be near 0.06 (0.08) for CALIOP all-RFV profiles. We further estimate a global mean aerosol extinction profile, a so-called noise floor, for CALIOP all-RFV profiles. The global mean CALIOP AOT is then recomputed by replacing RFV values with the derived noise-floor values for both all-RFV and non-all-RFV profiles. This process yields an improvement in the agreement of CALIOP and MODIS over-ocean AOT.

  20. Dust aerosol and optical properties over North Africa simulated with the ALADIN numerical prediction model from 2006 to 2010

    NASA Astrophysics Data System (ADS)

    Mokhtari, M.; Tulet, P.; Fischer, C.; Bouteloup, Y.; Bouyssel, F.; Brachemi, O.

    2015-02-01

    The seasonal cycle and optical properties of mineral dust aerosols in North Africa were simulated for the period from 2006 to 2010 using the numerical atmospheric model ALADIN coupled to the surface scheme SURFEX. The particularity of the simulations is that the major physical processes responsible for dust emission and transport, as well as radiative effects, are taken into account at short timescales and mesoscale resolution. The aim of these simulations is to quantify the dust emission and deposition, locate the major areas of dust emission and establish a climatology of aerosol optical properties in North Africa. The mean monthly Aerosol Optical Thickness (AOT) simulated by ALADIN is compared with the AOTs derived from the standard Dark Target (DT) and Deep Blue (DB) algorithms of the Aqua-MODIS (MODerate resolution Imaging Spectroradiometer) products over North Africa, and with a set of sun photometer measurements located at Banizoumbou, Cinzana, Soroa, Mbour and Capo Verde. The vertical distribution of dust aerosol represented by extinction profiles is also analysed using CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) observations. The annual dust emission simulated by ALADIN over North Africa is 878 Tg year-1. The Bodélé depression appears to be the main area of dust emission in North Africa, with an average estimate of about 21.6 Tg year-1. The simulated AOTs are in good agreement with satellite and sun photometer observations. The positions of the maxima of the modelled AOTs over North Africa match the observed positions, and the ALADIN simulations satisfactorily reproduce the various dust events over the 2006-2010 period. The AOT climatology proposed in this paper provides a solid database of optical properties and consolidates the existing climatology over this region derived from satellites, the AERONET network and Regional Climate Models. Moreover, the three-dimensional distribution of the simulated AOTs also provides information about the

  1. Two-Column Aerosol Project (TCAP) Field Campaign Report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Berg, Larry K

    This study included the deployment of the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility’s Mobile Facility (AMF), ARM Mobile Aerosol Observing System (MAOS) and the ARM Aerial Facility (AAF). The study was a collaborative effort involving scientists from DOE national laboratories, NOAA, NASA, and universities. The AAF and MAOS were deployed for two approximately month-long Intensive Operational Periods (IOPs) conducted in June 2012 and February 2013. Seasonal differences in the aerosol chemical and optical properties observed using the AMF, AAF, and MAOS are presented in this report. The total mass loading of aerosol is found tomore » be much greater in the summer than in the winter, with the difference associated with greater amounts of organic aerosol. The mass fraction of organic aerosol is much reduced in the winter, when sulfate is the dominant aerosol type. Surprisingly, very little sea-salt aerosol was observed in the summer. In contrast, much more sea salt aerosol was observed in the winter. The mass loading of black carbon is nearly the same in both seasons. These differences lead to a relative increase in the aerosol light absorption in the winter and an associated decrease in observed single-scattering albedo. Measurements of aerosol mixing state were made using a single-particle mass spectrometer, which showed that the majority of the summertime aerosol consisted of organic compounds mixed with various amounts of sulfate. A number of other findings are also summarized in the report, including: impact of aerosol layers aloft on the column aerosol optical depth; documentation of the aerosol properties at the AMF; differences in the aerosol properties associated with both columns, which are not systematic but reflect the complicated meteorological and chemical processes that impact aerosol as it is advected away from North America; and new instruments and data-processing techniques for measuring both

  2. Cloud and Aerosol Retrieval for the 2001 GLAS Satellite Lidar Mission

    NASA Technical Reports Server (NTRS)

    Hart, William D.; Palm, Stephen P.; Spinhirne, James D.

    2000-01-01

    The Geoscience Laser Altimeter System (GLAS) is scheduled for launch in July of 2001 aboard the Ice, Cloud and Land Elevation Satellite (ICESAT). In addition to being a precision altimeter for mapping the height of the Earth's icesheets, GLAS will be an atmospheric lidar, sensitive enough to detect gaseous, aerosol, and cloud backscatter signals, at horizontal and vertical resolutions of 175 and 75m, respectively. GLAS will be the first lidar to produce temporally continuous atmospheric backscatter profiles with nearly global coverage (94-degree orbital inclination). With a projected operational lifetime of five years, GLAS will collect approximately six billion lidar return profiles. The large volume of data dictates that operational analysis algorithms, which need to keep pace with the data yield of the instrument, must be efficient. So, we need to evaluate the ability of operational algorithms to detect atmospheric constituents that affect global climate. We have to quantify, in a statistical manner, the accuracy and precision of GLAS cloud and aerosol observations. Our poster presentation will show the results of modeling studies that are designed to reveal the effectiveness and sensitivity of GLAS in detecting various atmospheric cloud and aerosol features. The studies consist of analyzing simulated lidar returns. Simulation cases are constructed either from idealized renditions of atmospheric cloud and aerosol layers or from data obtained by the NASA ER-2 Cloud Lidar System (CLS). The fabricated renditions permit quantitative evaluations of operational algorithms to retrieve cloud and aerosol parameters. The use of observational data permits the evaluations of performance for actual atmospheric conditions. The intended outcome of the presentation is that climatology community will be able to use the results of these studies to evaluate and quantify the impact of GLAS data upon atmospheric modeling efforts.

  3. Normalization and calibration of geostationary satellite radiances for the International Satellite Cloud Climatology Project

    NASA Technical Reports Server (NTRS)

    Desormeaux, Yves; Rossow, William B.; Brest, Christopher L.; Campbell, G. G.

    1993-01-01

    Procedures are described for normalizing the radiometric calibration of image radiances obtained from geostationary weather satellites that contributed data to the International Satellite Cloud Climatology Project. The key step is comparison of coincident and collocated measurements made by each satellite and the concurrent AVHRR on the 'afternoon' NOAA polar-orbiting weather satellite at the same viewing geometry. The results of this comparison allow transfer of the AVHRR absolute calibration, which has been established over the whole series, to the radiometers on the geostationary satellites. Results are given for Meteosat-2, 3, and 4, for GOES-5, 6, and 7, for GMS-2, 3, and 4 and for Insat-1B. The relative stability of the calibrations of these radiance data is estimated to be within +/- 3 percent; the uncertainty of the absolute calibrations is estimated to be less than 10 percent. The remaining uncertainties are at least two times smaller than for the original radiance data.

  4. The influence of aerosols and land-use type on NO2 satellite retrieval over China

    NASA Astrophysics Data System (ADS)

    Liu, Mengyao; Lin, Jintai; Boersma, Folkert; Eskes, Henk; Chimot, Julien

    2017-04-01

    Both aerosols and surface reflectance have a strong influence on the retrieval of NO2 tropospheric vertical column densities (VCDs), especially over China with its heavy aerosol loading and rapid changes in land-use type. However, satellite retrievals of NO2 VCDs usually do not explicitly account for aerosol optical effects and surface reflectance anisotropy (BRDF) that varies in space and time. We develop an improved algorithm to derive tropospheric AMFs and VCDs over China from the OMI instrument - POMINO and DOMINO. This method can also be applied to TropOMI NO2 retrievals in the future. With small pixels of TropOMI and higher probability of encountering clear-sky scenes, the influence of BRDF and aerosol interference becomes more important than for OMI. Daily aerosol information is taken from the GEOS-Chem chemistry transport model and the aerosol optical depth (AOD) is adjusted via MODIS AOD climatology. We take the MODIS MCD43C2 C5 product to account for BRDF effects. The relative altitude of NO2 and aerosols is critical factor influencing the NO2 retrieval. In order to evaluate the aerosol extinction profiles (AEP) of GEOS-Chem improve our algorithm, we compare the GEOS-Chem simulation with CALIOP and develop a CALIOP AEP climatology to regulate the model's AEP. This provides a new way to include aerosol information into the tracer gas retrieval for OMI and TropOMI. Preliminary results indicate that the model performs reasonably well in reproducing the AEP shape. However, it seems to overestimate aerosols under 2km and underestimate above. We find that relative humidity (RH) is an important factor influencing the AEP shape when comparing the model with observations. If we adjust the GEOS-Chem RH to CALIOP's RH, the correlations of their AEPs also improve. Besides, take advantage of our retrieval method, we executed sensitivity tests to analyze their influences on NO2 trend and spatiotemporal variations in retrieval. It' the first time to investigate

  5. Satellite Remote Sensing of Aerosol Forcing

    NASA Technical Reports Server (NTRS)

    Remer, Lorraine; Kaufman, Yoram; Ramaprasad, Jaya; Procopio, Aline; Levin, Zev

    1999-01-01

    The role of aerosol forcing remains one of the largest uncertainties in estimating man's impact on the global climate system. One school of thought suggests that remote sensing by satellite sensors will provide the data necessary to narrow these uncertainties. While satellite measurements of direct aerosol forcing appear to be straightforward, satellite measurements of aerosol indirect forcing will be more complicated. Pioneering studies identified indirect aerosol forcing using AVHRR data in the biomass burning regions of Brazil. We have expanded this analysis with AVHRR to include an additional year of data and assimilated water vapor fields. The results show similar latitudinal dependence as reported by Kaufman and Fraser, but by using water vapor observations we conclude that latitude is not a proxy for water vapor and the strength of the indirect effect is not correlated to water vapor amounts. In addition to the AVHRR study we have identified indirect aerosol forcing in Brazil at much smaller spatial scales using the MODIS Airborne Simulator. The strength of the indirect effect appears to be related to cloud type and cloud dynamics. There is a suggestion that some of the cloud dynamics may be influenced by smoke destabilization of the atmospheric column. Finally, this study attempts to quantify remote sensing limitations due to the accuracy limits of the retrieval algorithms. We use a combination of numerical aerosol transport models, ground-based AERONET data and ISCCP cloud climatology to determine how much of the forcing occurs in regions too clean to determine from satellite retrievals.

  6. Aerosol Complexity and Implications for Predictability and Short-Term Forecasting

    NASA Technical Reports Server (NTRS)

    Colarco, Peter

    2016-01-01

    There are clear NWP and climate impacts from including aerosol radiative and cloud interactions. Changes in dynamics and cloud fields affect aerosol lifecycle, plume height, long-range transport, overall forcing of the climate system, etc. Inclusion of aerosols in NWP systems has benefit to surface field biases (e.g., T2m, U10m). Including aerosol affects has impact on analysis increments and can have statistically significant impacts on, e.g., tropical cyclogenesis. Above points are made especially with respect to aerosol radiative interactions, but aerosol-cloud interaction is a bigger signal on the global system. Many of these impacts are realized even in models with relatively simple (bulk) aerosol schemes (approx.10 -20 tracers). Simple schemes though imply simple representation of aerosol absorption and importantly for aerosol-cloud interaction particle-size distribution. Even so, more complex schemes exhibit a lot of diversity between different models, with issues such as size selection both for emitted particles and for modes. Prospects for complex sectional schemes to tune modal (and even bulk) schemes toward better selection of size representation. I think this is a ripe topic for more research -Systematic documentation of benefits of no vs. climatological vs. interactive (direct and then direct+indirect) aerosols. Document aerosol impact on analysis increments, inclusion in NWP data assimilation operator -Further refinement of baseline assumptions in model design (e.g., absorption, particle size distribution). Did not get into model resolution and interplay of other physical processes with aerosols (e.g., moist physics, obviously important), chemistry

  7. The direct effect of aerosols on solar radiation over the broader Mediterranean basin

    NASA Astrophysics Data System (ADS)

    Papadimas, C. D.; Hatzianastassiou, N.; Matsoukas, C.; Kanakidou, M.; Mihalopoulos, N.; Vardavas, I.

    2011-11-01

    For the first time, the direct radiative effect (DRE) of aerosols on solar radiation is computed over the entire Mediterranean basin, one of the most climatically sensitive world regions, by using a deterministic spectral radiation transfer model (RTM). The DRE effects on the outgoing shortwave radiation at the top of atmosphere (TOA), DRETOA, on the absorption of solar radiation in the atmospheric column, DREatm, and on the downward and absorbed surface solar radiation (SSR), DREsurf and DREnetsurf, respectively, are computed separately. The model uses input data for the period 2000-2007 for various surface and atmospheric parameters, taken from satellite (International Satellite Cloud Climatology Project, ISCCP-D2), Global Reanalysis projects (National Centers for Environmental Prediction - National Center for Atmospheric Research, NCEP/NCAR), and other global databases. The spectral aerosol optical properties (aerosol optical depth, AOD, asymmetry parameter, gaer and single scattering albedo, ωaer), are taken from the MODerate resolution Imaging Spectroradiometer (MODIS) of NASA (National Aeronautics and Space Administration) and they are Supplemented by the Global Aerosol Data Set (GADS). The model SSR fluxes have been successfully validated against measurements from 80 surface stations of the Global Energy Balance Archive (GEBA) covering the period 2000-2007. A planetary cooling is found above the Mediterranean on an annual basis (regional mean DRETOA = -2.4 Wm-2). Though planetary cooling is found over most of the region, up to -7 Wm-2, large positive DRETOA values (up to +25 Wm-2) are found over North Africa, indicating a strong planetary warming, as well as over the Alps (+0.5 Wm-2). Aerosols are found to increase the absorption of solar radiation in the atmospheric column over the region (DREatm = +11.1 Wm-2) and to decrease SSR (DREsurf = -16.5 Wm-2 and DREnetsurf -13.5 Wm-2) inducing thus significant atmospheric warming and surface radiative cooling

  8. EARLINET: towards an advanced sustainable European aerosol lidar network

    NASA Astrophysics Data System (ADS)

    Pappalardo, G.; Amodeo, A.; Apituley, A.; Comeron, A.; Freudenthaler, V.; Linné, H.; Ansmann, A.; Bösenberg, J.; D'Amico, G.; Mattis, I.; Mona, L.; Wandinger, U.; Amiridis, V.; Alados-Arboledas, L.; Nicolae, D.; Wiegner, M.

    2014-08-01

    The European Aerosol Research Lidar Network, EARLINET, was founded in 2000 as a research project for establishing a quantitative, comprehensive, and statistically significant database for the horizontal, vertical, and temporal distribution of aerosols on a continental scale. Since then EARLINET has continued to provide the most extensive collection of ground-based data for the aerosol vertical distribution over Europe. This paper gives an overview of the network's main developments since 2000 and introduces the dedicated EARLINET special issue, which reports on the present innovative and comprehensive technical solutions and scientific results related to the use of advanced lidar remote sensing techniques for the study of aerosol properties as developed within the network in the last 13 years. Since 2000, EARLINET has developed greatly in terms of number of stations and spatial distribution: from 17 stations in 10 countries in 2000 to 27 stations in 16 countries in 2013. EARLINET has developed greatly also in terms of technological advances with the spread of advanced multiwavelength Raman lidar stations in Europe. The developments for the quality assurance strategy, the optimization of instruments and data processing, and the dissemination of data have contributed to a significant improvement of the network towards a more sustainable observing system, with an increase in the observing capability and a reduction of operational costs. Consequently, EARLINET data have already been extensively used for many climatological studies, long-range transport events, Saharan dust outbreaks, plumes from volcanic eruptions, and for model evaluation and satellite data validation and integration. Future plans are aimed at continuous measurements and near-real-time data delivery in close cooperation with other ground-based networks, such as in the ACTRIS (Aerosols, Clouds, and Trace gases Research InfraStructure Network) www.actris.net, and with the

  9. Non-chemistry coupled PM10 modeling in Chiang Mai City, Northern Thailand: A fast operational approach for aerosol forecasts

    NASA Astrophysics Data System (ADS)

    Macatangay, Ronald; Bagtasa, Gerry; Sonkaew, Thiranan

    2017-09-01

    The Weather Research and Forecasting (WRF v. 3.7) model was applied to model PM10 data in Chiang Mai city for 10-days during a high haze event utilizing updated land use categories from the Moderate Resolution Imaging Spectroradiometer (MODIS). A higher resolution meteorological lateral boundary condition (from 1 degree to 0.25 degree) was also used from the NCEP GDAS/FNL Global Tropospheric Analyses and Forecast Grid system. A 3-category urban canopy model was also added and the Thompson aerosol-aware microphysics parameterization scheme was used to model the aerosol number concentrations that were later converted to PM10 concentrations. Aerosol number concentration monthly climatology was firstly used as initial and lateral boundary conditions to model PM10 concentrations. These were compared to surface data obtained from two stations of the Pollution Control Department (PCD) of Thailand. The results from the modeled PM10 concentrations could not capture the variability (r = 0.29; 0.27 for each site) and underestimated a high PM10 spike during the period studied. The authors then added satellite data to the aerosol climatology that improved the comparison with observations (r = 0.45; 43). However, both model runs still were not able to capture the high PM10 concentration event. This requires further investigation.

  10. Remote sensing of soot carbon - Part 1: Distinguishing different absorbing aerosol species

    NASA Astrophysics Data System (ADS)

    Schuster, G. L.; Dubovik, O.; Arola, A.

    2016-02-01

    We describe a method of using the Aerosol Robotic Network (AERONET) size distributions and complex refractive indices to retrieve the relative proportion of carbonaceous aerosols and free iron minerals (hematite and goethite). We assume that soot carbon has a spectrally flat refractive index and enhanced imaginary indices at the 440 nm wavelength are caused by brown carbon or hematite. Carbonaceous aerosols can be separated from dust in imaginary refractive index space because 95 % of biomass burning aerosols have imaginary indices greater than 0.0042 at the 675-1020 nm wavelengths, and 95 % of dust has imaginary refractive indices of less than 0.0042 at those wavelengths. However, mixtures of these two types of particles can not be unambiguously partitioned on the basis of optical properties alone, so we also separate these particles by size. Regional and seasonal results are consistent with expectations. Monthly climatologies of fine mode soot carbon are less than 1.0 % by volume for West Africa and the Middle East, but the southern African and South American biomass burning sites have peak values of 3.0 and 1.7 %. Monthly averaged fine mode brown carbon volume fractions have a peak value of 5.8 % for West Africa, 2.1 % for the Middle East, 3.7 % for southern Africa, and 5.7 % for South America. Monthly climatologies of free iron volume fractions show little seasonal variability, and range from about 1.1 to 1.7 % for coarse mode aerosols in all four study regions. Finally, our sensitivity study indicates that the soot carbon retrieval is not sensitive to the component refractive indices or densities assumed for carbonaceous and free iron aerosols, and the retrieval differs by only 15.4 % when these parameters are altered from our chosen baseline values. The total uncertainty of retrieving soot carbon mass is ˜ 50 % (when uncertainty in the AERONET product and mixing state is included in the analysis).

  11. The Sectional Stratospheric Sulfate Aerosol module (S3A-v1) within the LMDZ general circulation model: description and evaluation against stratospheric aerosol observations

    NASA Astrophysics Data System (ADS)

    Kleinschmitt, Christoph; Boucher, Olivier; Bekki, Slimane; Lott, François; Platt, Ulrich

    2017-09-01

    Stratospheric aerosols play an important role in the climate system by affecting the Earth's radiative budget as well as atmospheric chemistry, and the capabilities to simulate them interactively within global models are continuously improving. It is important to represent accurately both aerosol microphysical and atmospheric dynamical processes because together they affect the size distribution and the residence time of the aerosol particles in the stratosphere. The newly developed LMDZ-S3A model presented in this article uses a sectional approach for sulfate particles in the stratosphere and includes the relevant microphysical processes. It allows full interaction between aerosol radiative effects (e.g. radiative heating) and atmospheric dynamics, including e.g. an internally generated quasi-biennial oscillation (QBO) in the stratosphere. Sulfur chemistry is semi-prescribed via climatological lifetimes. LMDZ-S3A reasonably reproduces aerosol observations in periods of low (background) and high (volcanic) stratospheric sulfate loading, but tends to overestimate the number of small particles and to underestimate the number of large particles. Thus, it may serve as a tool to study the climate impacts of volcanic eruptions, as well as the deliberate anthropogenic injection of aerosols into the stratosphere, which has been proposed as a method of geoengineering to abate global warming.

  12. The Global Aerosol Synthesis and Science Project (GASSP): Measurements and Modeling to Reduce Uncertainty

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Reddington, C. L.; Carslaw, K. S.; Stier, P.

    The largest uncertainty in the historical radiative forcing of climate is caused by changes in aerosol particles due to anthropogenic activity. Sophisticated aerosol microphysics processes have been included in many climate models in an effort to reduce the uncertainty. However, the models are very challenging to evaluate and constrain because they require extensive in situ measurements of the particle size distribution, number concentration, and chemical composition that are not available from global satellite observations. The Global Aerosol Synthesis and Science Project (GASSP) aims to improve the robustness of global aerosol models by combining new methodologies for quantifying model uncertainty, tomore » create an extensive global dataset of aerosol in situ microphysical and chemical measurements, and to develop new ways to assess the uncertainty associated with comparing sparse point measurements with low-resolution models. GASSP has assembled over 45,000 hours of measurements from ships and aircraft as well as data from over 350 ground stations. The measurements have been harmonized into a standardized format that is easily used by modelers and nonspecialist users. Available measurements are extensive, but they are biased to polluted regions of the Northern Hemisphere, leaving large pristine regions and many continental areas poorly sampled. The aerosol radiative forcing uncertainty can be reduced using a rigorous model–data synthesis approach. Nevertheless, our research highlights significant remaining challenges because of the difficulty of constraining many interwoven model uncertainties simultaneously. Although the physical realism of global aerosol models still needs to be improved, the uncertainty in aerosol radiative forcing will be reduced most effectively by systematically and rigorously constraining the models using extensive syntheses of measurements.« less

  13. The Global Aerosol Synthesis and Science Project (GASSP): Measurements and Modeling to Reduce Uncertainty

    DOE PAGES

    Reddington, C. L.; Carslaw, K. S.; Stier, P.; ...

    2017-09-01

    The largest uncertainty in the historical radiative forcing of climate is caused by changes in aerosol particles due to anthropogenic activity. Sophisticated aerosol microphysics processes have been included in many climate models in an effort to reduce the uncertainty. However, the models are very challenging to evaluate and constrain because they require extensive in situ measurements of the particle size distribution, number concentration, and chemical composition that are not available from global satellite observations. The Global Aerosol Synthesis and Science Project (GASSP) aims to improve the robustness of global aerosol models by combining new methodologies for quantifying model uncertainty, tomore » create an extensive global dataset of aerosol in situ microphysical and chemical measurements, and to develop new ways to assess the uncertainty associated with comparing sparse point measurements with low-resolution models. GASSP has assembled over 45,000 hours of measurements from ships and aircraft as well as data from over 350 ground stations. The measurements have been harmonized into a standardized format that is easily used by modelers and nonspecialist users. Available measurements are extensive, but they are biased to polluted regions of the Northern Hemisphere, leaving large pristine regions and many continental areas poorly sampled. The aerosol radiative forcing uncertainty can be reduced using a rigorous model–data synthesis approach. Nevertheless, our research highlights significant remaining challenges because of the difficulty of constraining many interwoven model uncertainties simultaneously. Although the physical realism of global aerosol models still needs to be improved, the uncertainty in aerosol radiative forcing will be reduced most effectively by systematically and rigorously constraining the models using extensive syntheses of measurements.« less

  14. Measurement-based climatology of aerosol direct radiative effect, its sensitivities, and uncertainties from a background southeast US site

    NASA Astrophysics Data System (ADS)

    Sherman, James P.; McComiskey, Allison

    2018-03-01

    Aerosol optical properties measured at Appalachian State University's co-located NASA AERONET and NOAA ESRL aerosol network monitoring sites over a nearly four-year period (June 2012-Feb 2016) are used, along with satellite-based surface reflectance measurements, to study the seasonal variability of diurnally averaged clear sky aerosol direct radiative effect (DRE) and radiative efficiency (RE) at the top-of-atmosphere (TOA) and at the surface. Aerosol chemistry and loading at the Appalachian State site are likely representative of the background southeast US (SE US), home to high summertime aerosol loading and one of only a few regions not to have warmed during the 20th century. This study is the first multi-year ground truth DRE study in the SE US, using aerosol network data products that are often used to validate satellite-based aerosol retrievals. The study is also the first in the SE US to quantify DRE uncertainties and sensitivities to aerosol optical properties and surface reflectance, including their seasonal dependence.Median DRE for the study period is -2.9 W m-2 at the TOA and -6.1 W m-2 at the surface. Monthly median and monthly mean DRE at the TOA (surface) are -1 to -2 W m-2 (-2 to -3 W m-2) during winter months and -5 to -6 W m-2 (-10 W m-2) during summer months. The DRE cycles follow the annual cycle of aerosol optical depth (AOD), which is 9 to 10 times larger in summer than in winter. Aerosol RE is anti-correlated with DRE, with winter values 1.5 to 2 times more negative than summer values. Due to the large seasonal dependence of aerosol DRE and RE, we quantify the sensitivity of DRE to aerosol optical properties and surface reflectance, using a calendar day representative of each season (21 December for winter; 21 March for spring, 21 June for summer, and 21 September for fall). We use these sensitivities along with measurement uncertainties of aerosol optical properties and surface reflectance to calculate DRE uncertainties. We also

  15. Explicit and Observation-based Aerosol Treatment in Tropospheric NO2 Retrieval over China from the Ozone Monitoring Instrument

    NASA Astrophysics Data System (ADS)

    Liu, M.; Lin, J.; Boersma, F.; Pinardi, G.; Wang, Y.; Chimot, J.; Wagner, T.; Xie, P.; Eskes, H.; Van Roozendael, M.; Hendrick, F.

    2017-12-01

    Satellite retrieval of vertical column densities (VCDs) of tropospheric nitrogen dioxide (NO2) is influenced by aerosols substantially. Aerosols affect the retrieval of "effective cloud fraction (CF)" and "effective cloud top pressure (CP)" that are used in the subsequent NO2 retrieval to account for the presentence of clouds. And aerosol properties and vertical distributions directly affect the NO2 air mass factor (AMF) calculations. Our published POMINO algorithm uses a parallelized LIDORT-driven AMFv6 code to derive CF, CP and NO2 VCD. Daily information on aerosol optical properties are taken from GEOS-Chem simulations, with aerosol optical depth (AOD) further constrained by monthly MODIS AOD. However, the published algorithm does not include an observation-based constraint of aerosol vertical distribution. Here we construct a monthly climatological observation dataset of aerosol extinction profiles, based on Level-2 CALIOP data over 2007-2015, to further constrain aerosol vertical distributions. GEOS-Chem captures the temporal variations of CALIOP aerosol layer heights (ALH) but has an overall underestimate by about 0.3 km. It tends to overestimate the aerosol extinction by 10% below 2 km but with an underestimate by 30% above 2 km, leading to a low bias by 10-30% in the retrieved tropospheric NO2 VCD. After adjusting GEOS-Chem aerosol extinction profiles by the CALIOP monthly ALH climatology, the retrieved NO2 VCDs increase by 4-16% over China on a monthly basis in 2012. The improved NO2 VCDs are better correlated to independent MAX-DOAS observations at three sites than POMINO and DOMINO are - especially for the polluted cases, R2 reaches 0.76 for the adjusted POMINO, much higher than that for the published POMINO (0.68) and DOMINO (0.38). The newly retrieved CP increases by 60 hPa on average, because of a stronger aerosol screening effect. Compared to the CF used in DOMINO, which implicitly includes aerosol information, our improved CF is much lower and can

  16. Aerosol Measurements by the Globally Distributed Micro Pulse Lidar Network

    NASA Technical Reports Server (NTRS)

    Spinhirne, James; Welton, Judd; Campbell, James; Berkoff, Tim; Starr, David (Technical Monitor)

    2001-01-01

    Full time measurements of the vertical distribution of aerosol are now being acquired at a number of globally distributed MP (micro pulse) lidar sites. The MP lidar systems provide full time profiling of all significant cloud and aerosol to the limit of signal attenuation from compact, eye safe instruments. There are currently eight sites in operation and over a dozen planned. At all sited there are also passive aerosol and radiation measurements supporting the lidar data. Four of the installations are at Atmospheric Radiation Measurement program sites. The network operation includes instrument operation and calibration and the processing of aerosol measurements with standard retrievals and data products from the network sites. Data products include optical thickness and extinction cross section profiles. Application of data is to supplement satellite aerosol measurements and to provide a climatology of the height distribution of aerosol. The height distribution of aerosol is important for aerosol transport and the direct scattering and absorption of shortwave radiation in the atmosphere. Current satellite and other data already provide a great amount of information on aerosol distribution, but no passive technique can adequately resolve the height profile of aerosol. The Geoscience Laser Altimeter System (GLAS) is an orbital lidar to be launched in early 2002. GLAS will provide global measurements of the height distribution of aerosol. The MP lidar network will provide ground truth and analysis support for GLAS and other NASA Earth Observing System data. The instruments, sites, calibration procedures and standard data product algorithms for the MPL network will be described.

  17. Projected effect of 2000-2050 changes in climate and emissions on aerosol levels in China and associated transboundary transport

    EPA Science Inventory

    We investigate projected 2000–2050 changes in concentrations of aerosols in China and the associated transboundary aerosol transport by using the chemical transport model GEOS-Chem driven by the Goddard Institute for Space Studies (GISS) general circulation model (GCM) 3 at 4° × ...

  18. Radiative and temperature effects of aerosol simulated by the COSMO-Ru model for different atmospheric conditions and their testing against ground-based measurements and accurate RT simulations

    NASA Astrophysics Data System (ADS)

    Chubarova, Nataly; Poliukhov, Alexei; Shatunova, Marina; Rivin, Gdali; Becker, Ralf; Muskatel, Harel; Blahak, Ulrich; Kinne, Stefan; Tarasova, Tatiana

    2017-04-01

    We use the operational Russian COSMO-Ru weather forecast model (Ritter and and Geleyn, 1991) with different aerosol input data for the evaluation of radiative and temperature effects of aerosol in different atmospheric conditions. Various aerosol datasets were utilized including Tegen climatology (Tegen et al., 1997), updated Macv2 climatology (Kinne et al., 2013), Tanre climatology (Tanre et al., 1984) as well as the MACC data (Morcrette et al., 2009). For clear sky conditions we compare the radiative effects from the COSMO-Ru model over Moscow (55.7N, 37.5E) and Lindenberg/Falkenberg sites (52.2N, 14.1E) with the results obtained using long-term aerosol measurements. Additional tests of the COSMO RT code were performed against (FC05)-SW model (Tarasova T.A. and Fomin B.A., 2007). The overestimation of about 5-8% of COSMO RT code was obtained. The study of aerosol effect on temperature at 2 meters has revealed the sensitivity of about 0.7-1.1 degree C per 100 W/m2 change in shortwave net radiation due to aerosol variations. We also discuss the radiative impact of urban aerosol properties according to the long-term AERONET measurements in Moscow and Moscow suburb as well as long-term aerosol trends over Moscow from the measurements and Macv2 dataset. References: Kinne, S., O'Donnel D., Stier P., et al., J. Adv. Model. Earth Syst., 5, 704-740, 2013. Morcrette J.-J.,O. Boucher, L. Jones, eet al, J.GEOPHYS. RES.,VOL. 114, D06206, doi:10.1029/2008JD011235, 2009. Ritter, B. and Geleyn, J., Monthly Weather Review, 120, 303-325, 1992. Tanre, D., Geleyn, J., and Slingo, J., A. Deepak Publ., Hampton, Virginia, 133-177, 1984. Tarasova, T., and Fomin, B., Journal of Atmospheric and Oceanic Technology, 24, 1157-1162, 2007. Tegen, I., Hollrig, P., Chin, M., et al., Journal of Geophysical Research- Atmospheres, 102, 23895-23915, 1997.

  19. Comparing MODIS C6 'Deep Blue' and 'Dark Target' Aerosol Data

    NASA Technical Reports Server (NTRS)

    Hsu, N. C.; Sayer, A. M.; Bettenhausen, C.; Lee, J.; Levy, R. C.; Mattoo, S.; Munchak, L. A.; Kleidman, R.

    2014-01-01

    The MODIS Collection 6 Atmospheres product suite includes refined versions of both 'Deep Blue' (DB) and 'Dark Target' (DT) aerosol algorithms, with the DB dataset now expanded to include coverage over vegetated land surfaces. This means that, over much of the global land surface, users will have both DB and DT data to choose from. A 'merged' dataset is also provided, primarily for visualization purposes, which takes retrievals from either or both algorithms based on regional and seasonal climatologies of normalized difference vegetation index (NDVI). This poster present some comparisons of these two C6 aerosol algorithms, focusing on AOD at 550 nm derived from MODIS Aqua measurements, with each other and with Aerosol Robotic Network (AERONET) data, with the intent to facilitate user decisions about the suitability of the two datasets for their desired applications.

  20. Multiangle Imaging Spectroradiometer (MISR) Global Aerosol Optical Depth Validation Based on 2 Years of Coincident Aerosol Robotic Network (AERONET) Observations

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.; Gaitley, Barbara J.; Martonchik, John V.; Diner, David J.; Crean, Kathleen A.; Holben, Brent

    2005-01-01

    Performance of the Multiangle Imaging Spectroradiometer (MISR) early postlaunch aerosol optical thickness (AOT) retrieval algorithm is assessed quantitatively over land and ocean by comparison with a 2-year measurement record of globally distributed AERONET Sun photometers. There are sufficient coincident observations to stratify the data set by season and expected aerosol type. In addition to reporting uncertainty envelopes, we identify trends and outliers, and investigate their likely causes, with the aim of refining algorithm performance. Overall, about 2/3 of the MISR-retrieved AOT values fall within [0.05 or 20% x AOT] of Aerosol Robotic Network (AERONET). More than a third are within [0.03 or 10% x AOT]. Correlation coefficients are highest for maritime stations (approx.0.9), and lowest for dusty sites (more than approx.0.7). Retrieved spectral slopes closely match Sun photometer values for Biomass burning and continental aerosol types. Detailed comparisons suggest that adding to the algorithm climatology more absorbing spherical particles, more realistic dust analogs, and a richer selection of multimodal aerosol mixtures would reduce the remaining discrepancies for MISR retrievals over land; in addition, refining instrument low-light-level calibration could reduce or eliminate a small but systematic offset in maritime AOT values. On the basis of cases for which current particle models are representative, a second-generation MISR aerosol retrieval algorithm incorporating these improvements could provide AOT accuracy unprecedented for a spaceborne technique.

  1. The Southeastern Aerosol Research and Characterization (SEARCH) study: spatial variations and chemical climatology, 1999-2010.

    PubMed

    Blanchard, C L; Hidy, G M; Tanenbaum, S; Edgerton, E S; Hartsell, B E

    2013-03-01

    The Southeastern Aerosol Research and Characterization (SEARCH) study, which has been in continuous operation from 1999 to 2012, was implemented to investigate regional and urban air pollution in the southeastern United States. With complementary data from other networks, the SEARCH measurements provide key knowledge about long-term urban/nonurban pollution contrasts and regional climatology affecting inland locations and sites along the Gulf of Mexico coastline. Analytical approaches ranging from comparisons of mean concentrations to the application of air mass trajectories and principal component analysis provide insight into local and area-wide pollution. Gases (carbon monoxide, sulfur dioxide, nitrogen oxides, ozone, and ammonia), fine particle mass concentration, and fine particle species concentrations (including sulfate, elementary carbon, and organic carbon) are affected by a combination of regional conditions and local emission sources. Urban concentrations in excess of regional baselines and intraurban variations of concentrations depend on source proximity, topography, and local meteorological processes. Regional-scale pollution events (95th percentile concentrations) involving more than 6 of the 8 SEARCH sites are rare (< 2% of days), while subregional events affecting 4-6 sites occur on approximately 10% of days. Regional and subregional events are characterized by widely coincident elevated concentrations of ozone, sulfate, and particulate organic carbon, driven by persistent synoptic-scale air mass stagnation and higher temperatures that favor formation of secondary species, mainly in the summer months. The meteorological conditions associated with regional stagnation do not favor long-range transport of polluted air masses during episodes. Regional and subregional pollution events frequently terminate with southward and eastward penetration of frontal systems, which may initially reduce air pollutant concentrations more inland than along the Gulf

  2. Climatology of the Aerosol Optical Depth by Components from the Multi-Angle Imaging Spectroradiometer (MISR) and Chemistry Transport Models

    NASA Technical Reports Server (NTRS)

    Lee, Huikyo; Kalashnikova, Olga V.; Suzuki, Kentaroh; Braverman, Amy; Garay, Michael J.; Kahn, Ralph A.

    2016-01-01

    The Multi-angle Imaging Spectroradiometer (MISR) Joint Aerosol (JOINT_AS) Level 3 product has provided a global, descriptive summary of MISR Level 2 aerosol optical depth (AOD) and aerosol type information for each month over 16+ years since March 2000. Using Version 1 of JOINT_AS, which is based on the operational (Version 22) MISR Level 2 aerosol product, this study analyzes, for the first time, characteristics of observed and simulated distributions of AOD for three broad classes of aerosols: spherical nonabsorbing, spherical absorbing, and nonspherical - near or downwind of their major source regions. The statistical moments (means, standard deviations, and skew-nesses) and distributions of AOD by components derived from the JOINT_AS are compared with results from two chemistry transport models (CTMs), the Goddard Chemistry Aerosol Radiation and Transport (GOCART) and SPectral RadIatioN-TrAnSport (SPRINTARS). Overall, the AOD distributions retrieved from MISR and modeled by GOCART and SPRINTARS agree with each other in a qualitative sense. Marginal distributions of AOD for each aerosol type in both MISR and models show considerable high positive skewness, which indicates the importance of including extreme AOD events when comparing satellite retrievals with models. The MISR JOINT_AS product will greatly facilitate comparisons between satellite observations and model simulations of aerosols by type.

  3. Radiative Impact of Observed and Simulated Aerosol Layers Over the East Coast of North America

    NASA Astrophysics Data System (ADS)

    Berg, L. K.; Fast, J. D.; Burton, S. P.; Chand, D.; Comstock, J. M.; Ferrare, R. A.; Hair, J. W.; Hostetler, C. A.; Hubbe, J. M.; Kassianov, E.; Rogers, R. R.; Sedlacek, A. J., III; Shilling, J. E.; Tomlinson, J. M.; Wilson, J. M.; Zelenyuk, A.

    2014-12-01

    The vertical distribution of particles in the atmospheric column can have a large impact on the radiative forcing and cloud microphysics. A recent climatology constructed using data collected by the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) suggests elevated layers of aerosol are quite common near the North American east coast during both winter and summer. The Two-Column Aerosol Project (TCAP), conducted from June 2012 through June 2013, was a unique study utilizing both in situ and remotely sensed measurements designed to provide a comprehensive data set that can be used to investigate science questions related to aerosol radiative forcing and the vertical distribution of aerosol. The study sampled the atmosphere at a number of altitudes within two atmospheric columns; one located near the coast of North America (over Cape Cod, MA) and a second over the Atlantic Ocean several hundred kilometers from the coast. TCAP included the yearlong deployment of the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) located at the base of the Cape Cod column, as well as summer and winter aircraft intensive observation periods (IOPs) using the ARM Aerial Facility. One important finding from the TCAP summer IOP is the relatively common occurrence (during four of the six nearly cloud-free flights) of elevated aerosol layers in both the Cape Cod and maritime columns that were detected using the nadir pointing second-generation NASA Langley Research Center High-Spectral Resolution Lidar (HSRL-2). These elevated layers contributed up to 60% of the total observed aerosol optical depth (AOD). Many of these layers were also intercepted by the aircraft configured for in situ sampling, and the aerosol in the layers was found to have increased amounts of biomass burning material and nitrate compared to aerosol found near the surface. Both the in situ and remote sensing observations have been compared to

  4. Volcanic-aerosol-induced changes in stratospheric ozone following the eruption of Mount Pinatubo

    NASA Technical Reports Server (NTRS)

    Grant, W. B.; Browell, E. V.; Fishman, J.; Brackett, V. G.; Fenn, M. A.; Butler, C. F.; Nganga, D.; Minga, A.; Cros, B.; Mayor, S. D.

    1994-01-01

    Measurements of lower stratospheric ozone in the Tropics using electrochemical concentrations cell (ECC) sondes and the airborne UV Differential Absorption Lidar (DIAL) system after the eruption of Mt. Pinatubo are compared with the Stratospheric Aerosol and Gas Experiment 2 (SAGE 2) and ECC sonde measurements from below the eruption to determine what changes have occurred as a result. Aerosol data from the Advanced Very High Resolution Radiometer (AVHRR) and the visible and IR wavelengths of the lidar system are used to examine the relationship between aerosols and ozone changes. Ozone decreases of 30 percent at altitudes between 19 and 26 km, partial column (16-28 km) decreases of about 27 D.U., and slight increases (5.4 D.U.) between 28 and 31 km are found in comparison with SAGE 2 climatological values.

  5. Joint Retrieval Of Surface Reflectance And Aerosol Properties: Application To MSG/SEVIRI in the framework of the aerosol_cci project

    NASA Astrophysics Data System (ADS)

    Luffarelli, Marta; Govaerts, Yves; Goossens, Cedric

    2017-04-01

    A new versatile algorithm for the joint retrieval of surface reflectance and aerosol properties has been developed and tested at Rayference. This algorithm, named Combined Inversion of Surface and Aerosols (CISAR), includes a fast physically-based Radiative Transfer Model (RTM) accounting for the surface reflectance anisotropy and its coupling with aerosol scattering. This RTM explicitly solves the radiative transfer equation during the inversion process, without relying on pre-calculated integrals stored in LUT, allowing for a continuous variation of the state variables in the solution space. The inversion is based on a Optimal Estimation (OE) approach, which seeks for the best balance between the information coming from the observation and the a priori information. The a priori information is any additional knowledge on the observed system and it can concern the magnitude of the state variable or constraints on temporal and spectral variability. Both observations and priori information are provided with the corresponding uncertainty. For each processed spectral band, CISAR delivers the surface Bidirectional Reflectance Factor (BRF) and aerosol optical thickness, discriminating the effects of small and large particles. It also provides the associated uncertainty covariance matrix for every processed pixels. In the framework of the ESA aerosol_cci project, CISAR is applied on TOA BRF acquired by SEVIRI onboard Meteosat Second Generation (MSG) in the VIS0.6, VIS0.8 and NIR1.6 spectral bands. SEVIRI observations are accumulated during several days to document the surface anisotropy and minimize the impact of clouds. While surface radiative properties are supposed constant during this accumulation period, aerosol properties are derived on an hourly basis. The information content of each MSG/SEVIRI band will be provided based on the analysis of the posterior uncertainty covariance matrix. The analysis will demonstrate in particular the capability of CISAR to decouple

  6. Aerosol Retrievals from ARM SGP MFRSR Data

    DOE Data Explorer

    Alexandrov, Mikhail

    2008-01-15

    The Multi-Filter Rotating Shadowband Radiometer (MFRSR) makes precise simultaneous measurements of the solar direct normal and diffuse horizontal irradiances at six wavelengths (nominally 415, 500, 615, 673, 870, and 940 nm) at short intervals (20 sec for ARM instruments) throughout the day. Time series of spectral optical depth are derived from these measurements. Besides water vapor at 940 nm, the other gaseous absorbers within the MFRSR channels are NO2 (at 415, 500, and 615 nm) and ozone (at 500, 615, and 670 nm). Aerosols and Rayleigh scattering contribute atmospheric extinction in all MFRSR channels. Our recently updated MFRSR data analysis algorithm allows us to partition the spectral aerosol optical depth into fine and coarse modes and to retrieve the fine mode effective radius. In this approach we rely on climatological amounts of NO2 from SCIAMACHY satellite retrievals and use daily ozone columns from TOMS.

  7. A Mesoscale Analysis of Column-Integrated Aerosol Properties in Northern India During the TIGERZ 2008 Pre-Monsoon Period and a Comparison to MODIS Retrievals

    NASA Technical Reports Server (NTRS)

    Giles, D. M.; Holben, B. N.; Tripathi, S. N.; Eck, T. F.; Newcomb, W. W.; Slutsker, I.; Dickerson, R. R.; Thompson, A. M.; Wang, S.-H.; Singh, R. P.; hide

    2010-01-01

    The Indo-Gangetic Plain (IGP) of the northern Indian subcontinent produces anthropogenic pollution from urban, industrial and rural combustion sources nearly continuously and is affected by convection-induced winds driving desert and alluvial dust into the atmosphere during the premonsoon period. Within the IGP, the NASA Aerosol Robotic Network (AERONET) project initiated the TIGERZ measurement campaign in May 2008 with an intensive operational period from May 1 to June 23, 2008. Mesoscale spatial variability of aerosol optical depth (AOD, tau) measurements at 500mn was assessed at sites around Kanpur, India, with averages ranging from 0.31 to 0.89 for spatial variability study (SVS) deployments. Sites located downwind from the city of Kanpur indicated slightly higher average aerosol optical depth (delta Tau(sub 500)=0.03-0.09). In addition, SVS AOD area-averages were compared to the long-tenn Kanpur AERONET site data: Four SVS area-averages were within +/- 1 cr of the climatological mean of the Kanpur site, while one SVS was within 2sigma below climatology. For a SVS case using AERONET inversions, the 440-870mn Angstrom exponent of approximately 0.38, the 440-870mn absorption Angstrom exponent (AAE) of 1.15-1.53, and the sphericity parameter near zero suggested the occurrence of large, strongly absorbing, non-spherical aerosols over Kanpur (e.g., mixed black carbon and dust) as well as stronger absorption downwind of Kanpur. Furthermore, the 3km and lOkm Terra and Aqua MODIS C005 aerosol retrieval algorithms at tau(sub 550) were compared to the TIGERZ data set. Although MODIS retrievals at higher quality levels were comparable to the MODIS retrieval uncertainty, the total number of MODIS matchups (N) were reduced with subsequent quality levels (N=25, QA>=0; N=9,QA>=l; N=6, QA>=2; N=1, QA=3) over Kanpur during the premonsoon primarily due to the semi-bright surface, complex aerosol mixture and cloud-contaminated pixels. The TIGERZ 2008 data set provided a unique

  8. Campaign datasets for Two-Column Aerosol Project (TCAP)

    DOE Data Explorer

    Berg,Larry; Mei,Fan; Cairns,Brian; Chand,Duli; Comstock,Jennifer; Cziczo,Daniel; Hostetler,Chris; Hubbe,John; Long,Chuck; Michalsky,Joseph; Pekour,Mikhail; Russell,Phil; Scott,Herman; Sedlacek,Arthur; Shilling,John; Springston,Stephen; Tomlinson,Jason; Watson,Thomas; Zelenyuk-Imre,Alla

    2013-12-30

    This campaign was designed to provide a detailed set of observations with which to 1) perform radiative and cloud condensation nuclei (CCN) closure studies, 2) evaluate a new retrieval algorithm for aerosol optical depth (AOD) in the presence of clouds using passive remote sensing 3) extend a previously developed technique to investigate aerosol indirect effects, and 4) evaluate the performance of a detailed regional-scale model and a more parameterized global-scale model in simulating particle activation and AOD associated with the aging of anthropogenic aerosols. To meet these science objectives, the ARM Mobile Facility (AMF) and the Mobile Aerosol Observing System (MAOS) was deployed on Cape Cod, Massachusetts for a 12-month period starting in the summer of 2012 in order to quantify aerosol properties, radiation and cloud characteristics at a location subject to both clear- and cloudy- conditions, and clean- and polluted-conditions. These observations were supplemented by two aircraft intensive observation periods (IOPS), one in the summer and a second in the winter. Each IOP required two aircraft.

  9. MACv2-SP: a parameterization of anthropogenic aerosol optical properties and an associated Twomey effect for use in CMIP6

    NASA Astrophysics Data System (ADS)

    Stevens, Bjorn; Fiedler, Stephanie; Kinne, Stefan; Peters, Karsten; Rast, Sebastian; Müsse, Jobst; Smith, Steven J.; Mauritsen, Thorsten

    2017-02-01

    A simple plume implementation of the second version (v2) of the Max Planck Institute Aerosol Climatology, MACv2-SP, is described. MACv2-SP provides a prescription of anthropogenic aerosol optical properties and an associated Twomey effect. It was created to provide a harmonized description of post-1850 anthropogenic aerosol radiative forcing for climate modeling studies. MACv2-SP has been designed to be easy to implement, change and use, and thereby enable studies exploring the climatic effects of different patterns of aerosol radiative forcing, including a Twomey effect. MACv2-SP is formulated in terms of nine spatial plumes associated with different major anthropogenic source regions. The shape of the plumes is fit to the Max Planck Institute Aerosol Climatology, version 2, whose present-day (2005) distribution is anchored by surface-based observations. Two types of plumes are considered: one predominantly associated with biomass burning, the other with industrial emissions. These differ in the prescription of their annual cycle and in their optical properties, thereby implicitly accounting for different contributions of absorbing aerosol to the different plumes. A Twomey effect for each plume is prescribed as a change in the host model's background cloud-droplet population density using relationships derived from satellite data. Year-to-year variations in the amplitude of the plumes over the historical period (1850-2016) are derived by scaling the plumes with associated national emission sources of SO2 and NH3. Experiments using MACv2-SP are performed with the Max Planck Institute Earth System Model. The globally and annually averaged instantaneous and effective aerosol radiative forcings are estimated to be -0.6 and -0.5 W m-2, respectively. Forcing from aerosol-cloud interactions (the Twomey effect) offsets the reduction of clear-sky forcing by clouds, so that the net effect of clouds on the aerosol forcing is small; hence, the clear-sky forcing, which is more

  10. Two-Column Aerosol Project (TCAP): Ground-Based Radiation and Aerosol Validation Using the NOAA Mobile SURFRAD Station Field Campaign Report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Michalsky, Joseph; Lantz, Kathy

    The National Oceanic and Atmospheric Administration (NOAA) is preparing for the launch of the Geostationary Operational Environmental Satellite R-Series (GOES-R) satellite in 2015. This satellite will feature higher time (5-minute versus 30-minute sampling) and spatial resolution (0.5 km vs 1 km in the visible channel) than current GOES instruments provide. NOAA’s National Environmental Satellite Data and Information Service has funded the Global Monitoring Division at the Earth System Research Laboratory to provide ground-based validation data for many of the new and old products the new GOES instruments will retrieve specifically related to radiation at the surface and aerosol and itsmore » extensive and intensive properties in the column. The Two-Column Aerosol Project (TCAP) had an emphasis on aerosol; therefore, we asked to be involved in this campaign to de-bug our new instrumentation and to provide a new capability that the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility’s Mobile Facilities (AMF) did not possess, namely surface albedo measurement out to 1625 nm. This gave us a chance to test remote operation of our new multi-filter rotating shadowband radiometer/multi-filter radiometer (MFRSR/MFR) combination. We did not deploy standard broadband shortwave and longwave radiation instrumentation because ARM does this as part of every AMF deployment. As it turned out, the ARM standard MFRSR had issues, and we were able to provide the aerosol column data for the first 2 months of the campaign covering the summer flight phase of the deployment. Using these data, we were able to work with personnel at Pacific Northwest National Laboratory (PNNL) to retrieve not only aerosol optical depth (AOD), but single scattering albedo and asymmetry parameter, as well.« less

  11. A global satellite assisted precipitation climatology

    USGS Publications Warehouse

    Funk, Christopher C.; Verdin, Andrew P.; Michaelsen, Joel C.; Pedreros, Diego; Husak, Gregory J.; Peterson, P.

    2015-01-01

    Accurate representations of mean climate conditions, especially in areas of complex terrain, are an important part of environmental monitoring systems. As high-resolution satellite monitoring information accumulates with the passage of time, it can be increasingly useful in efforts to better characterize the earth's mean climatology. Current state-of-the-science products rely on complex and sometimes unreliable relationships between elevation and station-based precipitation records, which can result in poor performance in food and water insecure regions with sparse observation networks. These vulnerable areas (like Ethiopia, Afghanistan, or Haiti) are often the critical regions for humanitarian drought monitoring. Here, we show that long period of record geo-synchronous and polar-orbiting satellite observations provide a unique new resource for producing high resolution (0.05°) global precipitation climatologies that perform reasonably well in data sparse regions. Traditionally, global climatologies have been produced by combining station observations and physiographic predictors like latitude, longitude, elevation, and slope. While such approaches can work well, especially in areas with reasonably dense observation networks, the fundamental relationship between physiographic variables and the target climate variables can often be indirect and spatially complex. Infrared and microwave satellite observations, on the other hand, directly monitor the earth's energy emissions. These emissions often correspond physically with the location and intensity of precipitation. We show that these relationships provide a good basis for building global climatologies. We also introduce a new geospatial modeling approach based on moving window regressions and inverse distance weighting interpolation. This approach combines satellite fields, gridded physiographic indicators, and in situ climate normals. The resulting global 0.05° monthly precipitation climatology, the Climate

  12. Regional-scale relationships between aerosol and summer monsoon circulation, and precipitation over northeast Asia

    NASA Astrophysics Data System (ADS)

    Yoon, Soon-Chang; Kim, Sang-Woo; Choi, Suk-Jin; Choi, In-Jin

    2010-08-01

    We investigated the regional-scale relationships between columnar aerosol loads and summer monsoon circulation, and also the precipitation over northeast Asia using aerosol optical depth (AOD) data obtained from the 8-year MODIS, AERONET Sun/sky radiometer, and precipitation data acquired under the Global Precipitation Climatology Project (GPCP). These high-quality data revealed the regional-scale link between AOD and summer monsoon circulation, precipitation in July over northeast Asian countries, and their distinct spatial and annual variabilities. Compared to the mean AOD for the entire period of 2001-2008, the increase of almost 40-50% in the AOD value in July 2005 and July 2007 was found over the downwind regions of China (Yellow Sea, Korean peninsula, and East Sea), with negative precipitation anomalies. This can be attributable to the strong westerly confluent flows, between cyclone flows by continental thermal low centered over the northern China and anticyclonic flows by the western North Pacific High, which transport anthropogenic pollution aerosols emitted from east China to aforementioned downwind high AOD regions along the rim of the Pacific marine airmass. In July 2002, however, the easterly flows transported anthropogenic aerosols from east China to the southwestern part of China in July 2002. As a result, the AOD off the coast of China was dramatically reduced in spite of decreasing rainfall. From the calculation of the cross-correlation coefficient between MODIS-derived AOD anomalies and GPCP precipitation anomalies in July over the period 2001-2008, we found negative correlations over the areas encompassed by 105-115°E and 30-35°N and by 120-140°E and 35-40°N (Yellow Sea, Korean peninsula, and East Sea). This suggests that aerosol loads over these regions are easily influenced by the Asian monsoon flow system and associated precipitation.

  13. SPARC Intercomparison of Middle Atmosphere Climatologies

    NASA Technical Reports Server (NTRS)

    Randel, William; Fleming, Eric; Geller, Marvin; Hamilton, Kevin; Karoly, David; Ortland, Dave; Pawson, Steve; Swinbank, Richard; Udelhofen, Petra

    2002-01-01

    This atlas presents detailed incomparisons of several climatological wind and temperature data sets which cover the middle atmosphere (over altitudes approx. 10-80 km). A number of middle atmosphere climatologies have been developed in the research community based on a variety of meteorological analyses and satellite data sets. Here we present comparisons between these climatological data sets for a number of basic circulation statistics, such as zonal mean temperature, winds and eddy flux statistics. Special attention is focused on tropical winds and temperatures, where large differences exist among separate analyses. We also include comparisons between the global climatologies and historical rocketsonde wind and temperature measurements, and also with more recent lidar temperature data. These comparisons highlight differences and uncertainties in contemporary middle atmosphere data sets, and allow biases in particular analyses to be isolated. In addition, a brief atlas of zonal mean temperature and wind statistics is provided to highlight data availability and as a quick-look reference. This technical report is intended as a companion to the climatological data sets held in archive at the SPARC Data Center (http://www.sparc.sunysb.edu).

  14. Simulation of tropospheric chemistry and aerosols with the climate model EC-Earth

    NASA Astrophysics Data System (ADS)

    van Noije, T. P. C.; Le Sager, P.; Segers, A. J.; van Velthoven, P. F. J.; Krol, M. C.; Hazeleger, W.

    2014-03-01

    We have integrated the atmospheric chemistry and transport model TM5 into the global climate model EC-Earth version 2.4. We present an overview of the TM5 model and the two-way data exchange between TM5 and the integrated forecasting system (IFS) model from the European Centre for Medium-Range Weather Forecasts (ECMWF), the atmospheric general circulation model of EC-Earth. In this paper we evaluate the simulation of tropospheric chemistry and aerosols in a one-way coupled configuration. We have carried out a decadal simulation for present-day conditions and calculated chemical budgets and climatologies of tracer concentrations and aerosol optical depth. For comparison we have also performed offline simulations driven by meteorological fields from ECMWF's ERA-Interim reanalysis and output from the EC-Earth model itself. Compared to the offline simulations, the online-coupled system produces more efficient vertical mixing in the troposphere, which likely reflects an improvement of the treatment of cumulus convection. The chemistry in the EC-Earth simulations is affected by the fact that the current version of EC-Earth produces a cold bias with too dry air in large parts of the troposphere. Compared to the ERA-Interim driven simulation, the oxidizing capacity in EC-Earth is lower in the tropics and higher in the extratropics. The methane lifetime is 7% higher in EC-Earth, but remains well within the range reported in the literature. We evaluate the model by comparing the simulated climatologies of surface carbon monoxide, tropospheric and surface ozone, and aerosol optical depth against observational data. The work presented in this study is the first step in the development of EC-Earth into an Earth system model with fully interactive atmospheric chemistry and aerosols.

  15. Simulation of tropospheric chemistry and aerosols with the climate model EC-Earth

    NASA Astrophysics Data System (ADS)

    van Noije, T. P. C.; Le Sager, P.; Segers, A. J.; van Velthoven, P. F. J.; Krol, M. C.; Hazeleger, W.; Williams, A. G.; Chambers, S. D.

    2014-10-01

    We have integrated the atmospheric chemistry and transport model TM5 into the global climate model EC-Earth version 2.4. We present an overview of the TM5 model and the two-way data exchange between TM5 and the IFS model from the European Centre for Medium-Range Weather Forecasts (ECMWF), the atmospheric general circulation model of EC-Earth. In this paper we evaluate the simulation of tropospheric chemistry and aerosols in a one-way coupled configuration. We have carried out a decadal simulation for present-day conditions and calculated chemical budgets and climatologies of tracer concentrations and aerosol optical depth. For comparison we have also performed offline simulations driven by meteorological fields from ECMWF's ERA-Interim reanalysis and output from the EC-Earth model itself. Compared to the offline simulations, the online-coupled system produces more efficient vertical mixing in the troposphere, which reflects an improvement of the treatment of cumulus convection. The chemistry in the EC-Earth simulations is affected by the fact that the current version of EC-Earth produces a cold bias with too dry air in large parts of the troposphere. Compared to the ERA-Interim driven simulation, the oxidizing capacity in EC-Earth is lower in the tropics and higher in the extratropics. The atmospheric lifetime of methane in EC-Earth is 9.4 years, which is 7% longer than the lifetime obtained with ERA-Interim but remains well within the range reported in the literature. We further evaluate the model by comparing the simulated climatologies of surface radon-222 and carbon monoxide, tropospheric and surface ozone, and aerosol optical depth against observational data. The work presented in this study is the first step in the development of EC-Earth into an Earth system model with fully interactive atmospheric chemistry and aerosols.

  16. Revisiting a Hydrological Analysis Framework with International Satellite Land Surface Climatology Project Initiative 2 Rainfall, Net Radiation, and Runoff Fields

    NASA Technical Reports Server (NTRS)

    Koster, Randal D.; Fekete, Balazs M.; Huffman, George J.; Stackhouse, Paul W.

    2006-01-01

    The International Satellite Land Surface Climatology Project Initiative 2 (ISLSCP-2) data set provides the data needed to characterize the surface water budget across much of the globe in terms of energy availability (net radiation) and water availability (precipitation) controls. The data, on average, are shown to be consistent with Budyko s decades-old framework, thereby demonstrating the continuing relevance of Budyko s semiempirical relationships. This consistency, however, appears only when a small subset of the data with hydrologically suspicious behavior is removed from the analysis. In general, the precipitation, net radiation, and runoff data also appear consistent in their interannual variability and in the phasing of their seasonal cycles.

  17. Spatio-temporal variability of aerosols in the tropics relationship with atmospheric and oceanic environments

    NASA Astrophysics Data System (ADS)

    Zuluaga-Arias, Manuel D.

    2011-12-01

    Earth's radiation budget is directly influenced by aerosols through the absorption of solar radiation and subsequent heating of the atmosphere. Aerosols modulate the hydrological cycle indirectly by modifying cloud properties, precipitation and ocean heat storage. In addition, polluting aerosols impose health risks in local, regional and global scales. In spite of recent advances in the study of aerosols variability, uncertainty in their spatio-temporal distributions still presents a challenge in the understanding of climate variability. For example, aerosol loading varies not only from year to year but also on higher frequency intraseasonal time scales producing strong variability on local and regional scales. An assessment of the impact of aerosol variability requires long period measurements of aerosols at both regional and global scales. The present dissertation compiles a large database of remotely sensed aerosol loading in order to analyze its spatio-temporal variability, and how this load interacts with different variables that characterize the dynamic and thermodynamic states of the environment. Aerosol Index (AI) and Aerosol Optical Depth (AOD) were used as measures of the atmospheric aerosol load. In addition, atmospheric and oceanic satellite observations, and reanalysis datasets is used in the analysis to investigate aerosol-environment interactions. A diagnostic study is conducted to produce global and regional aerosol satellite climatologies, and to analyze and compare the validity of aerosol retrievals. We find similarities and differences between the aerosol distributions over various regions of the globe when comparing the different satellite retrievals. A nonparametric approach is also used to examine the spatial distribution of the recent trends in aerosol concentration. A significant positive trend was found over the Middle East, Arabian Sea and South Asian regions strongly influenced by increases in dust events. Spectral and composite analyses

  18. Overview of ACE-Asia Spring 2001 Investigations on Aerosol Radiative Effects and Related Aerosol Properties

    NASA Technical Reports Server (NTRS)

    Russell, Philip B.; Valero, F. P. J.; Flatau, P. J.; Bergin, M.; Holben, B.; Nakajima, T.; Pilewskie, P.; Bergstrom, R.; Hipskind, R. Stephen (Technical Monitor)

    2001-01-01

    A primary, ACE-Asia objective was to quantify the interactions between aerosols and radiation in the Asia-Pacific region. Toward this end, radiometric and related aerosol measurements were made from ocean, land, air and space platforms. Models that predict aerosol fields guided the measurements and are helping integrate and interpret results. Companion overview's survey these measurement and modeling components. Here we illustrate how these components were combined to determine aerosol radiative. impacts and their relation to aerosol properties. Because clouds can obscure or change aerosol direct radiative effects, aircraft and ship sorties to measure these effects depended on predicting and finding cloud-free areas and times with interesting aerosols present. Pre-experiment satellite cloud climatologies, pre-flight aerosol and cloud forecasts, and in-flight guidance from satellite imagery all helped achieve this. Assessments of aerosol regional radiative impacts benefit from the spatiotemporal coverage of satellites, provided satellite-retrieved aerosol properties are accurate. Therefore, ACE-Asia included satellite retrieval tests, as part of many comparisons to judge the consistency (closure) among, diverse measurements. Early results include: (1) Solar spectrally resolved and broadband irradiances and optical depth measurements from the C-130 aircraft and at Kosan, Korea yielded aerosol radiative forcing efficiencies, permitting comparisons between efficiencies of ACE-Asia and INDOEX aerosols, and between dust and "pollution" aerosols. Detailed results will be presented in separate papers. (2) Based on measurements of wavelength dependent aerosol optical depth (AOD) and single scattering albedo the estimated 24-h a average aerosol radiative forcing efficiency at the surface for photosynthetically active radiation (400 - 700 nm) in Yulin, China is approx. 30 W sq m per AOD(500 nm). (3) The R/V Brown cruise from Honolulu to Sea of Japan sampled an aerosol optical

  19. CMIP5 models' shortwave cloud radiative response and climate sensitivity linked to the climatological Hadley cell extent

    NASA Astrophysics Data System (ADS)

    Lipat, Bernard R.; Tselioudis, George; Grise, Kevin M.; Polvani, Lorenzo M.

    2017-06-01

    This study analyzes Coupled Model Intercomparison Project phase 5 (CMIP5) model output to examine the covariability of interannual Southern Hemisphere Hadley cell (HC) edge latitude shifts and shortwave cloud radiative effect (SWCRE). In control climate runs, during years when the HC edge is anomalously poleward, most models substantially reduce the shortwave radiation reflected by clouds in the lower midlatitude region (LML; ˜28°S-˜48°S), although no such reduction is seen in observations. These biases in HC-SWCRE covariability are linked to biases in the climatological HC extent. Notably, models with excessively equatorward climatological HC extents have weaker climatological LML subsidence and exhibit larger increases in LML subsidence with poleward HC edge expansion. This behavior, based on control climate interannual variability, has important implications for the CO2-forced model response. In 4×CO2-forced runs, models with excessively equatorward climatological HC extents produce stronger SW cloud radiative warming in the LML region and tend to have larger climate sensitivity values than models with more realistic climatological HC extents.

  20. 30 CFR 779.18 - Climatological information.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 30 Mineral Resources 3 2012-07-01 2012-07-01 false Climatological information. 779.18 Section 779... PROGRAMS SURFACE MINING PERMIT APPLICATIONS-MINIMUM REQUIREMENTS FOR INFORMATION ON ENVIRONMENTAL RESOURCES § 779.18 Climatological information. (a) When requested by the regulatory authority, the application...

  1. 30 CFR 779.18 - Climatological information.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 30 Mineral Resources 3 2011-07-01 2011-07-01 false Climatological information. 779.18 Section 779... PROGRAMS SURFACE MINING PERMIT APPLICATIONS-MINIMUM REQUIREMENTS FOR INFORMATION ON ENVIRONMENTAL RESOURCES § 779.18 Climatological information. (a) When requested by the regulatory authority, the application...

  2. 30 CFR 783.18 - Climatological information.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 30 Mineral Resources 3 2012-07-01 2012-07-01 false Climatological information. 783.18 Section 783... PROGRAMS UNDERGROUND MINING PERMIT APPLICATIONS-MINIMUM REQUIREMENTS FOR INFORMATION ON ENVIRONMENTAL RESOURCES § 783.18 Climatological information. (a) When requested by the regulatory authority, the...

  3. 30 CFR 783.18 - Climatological information.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 30 Mineral Resources 3 2011-07-01 2011-07-01 false Climatological information. 783.18 Section 783... PROGRAMS UNDERGROUND MINING PERMIT APPLICATIONS-MINIMUM REQUIREMENTS FOR INFORMATION ON ENVIRONMENTAL RESOURCES § 783.18 Climatological information. (a) When requested by the regulatory authority, the...

  4. 16 year climatology of cirrus clouds over a tropical station in southern India using ground and space-based lidar observations

    NASA Astrophysics Data System (ADS)

    Pandit, A. K.; Gadhavi, H. S.; Venkat Ratnam, M.; Raghunath, K.; Rao, S. V. B.; Jayaraman, A.

    2015-06-01

    16 year (1998-2013) climatology of cirrus clouds and their macrophysical (base height, top height and geometrical thickness) and optical properties (cloud optical thickness) observed using a ground-based lidar over Gadanki (13.5° N, 79.2° E), India, is presented. The climatology obtained from the ground-based lidar is compared with the climatology obtained from seven and half years (June 2006-December 2013) of Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) observations. A very good agreement is found between the two climatologies in spite of their opposite viewing geometries and difference in sampling frequencies. Nearly 50-55% of cirrus clouds were found to possess geometrical thickness less than 2 km. Ground-based lidar is found to detect more number of sub-visible clouds than CALIOP which has implications for global warming studies as sub-visible cirrus clouds have significant positive radiative forcing. Cirrus clouds with mid-cloud temperatures between -50 to -70 °C have a mean geometrical thickness greater than 2 km in contrast to the earlier reported value of 1.7 km. Trend analyses reveal a statistically significant increase in the altitude of sub-visible cirrus clouds which is consistent with the recent climate model simulations. Also, the fraction of sub-visible cirrus cloud is found to be increasing during the last sixteen years (1998 to 2013) which has implications to the temperature and water vapour budget in the tropical tropopause layer.

  5. Improvements to the OMI Near-uv Aerosol Algorithm Using A-train CALIOP and AIRS Observations

    NASA Technical Reports Server (NTRS)

    Torres, O.; Ahn, C.; Zhong, C.

    2014-01-01

    The height of desert dust and carbonaceous aerosols layers and, to a lesser extent, the difficulty in assessing the predominant size mode of these absorbing aerosol types, are sources of uncertainty in the retrieval of aerosol properties from near UV satellite observations. The availability of independent, near-simultaneous measurements of aerosol layer height, and aerosol-type related parameters derived from observations by other A-train sensors, makes possible the direct use of these parameters as input to the OMI (Ozone Monitoring Instrument) near UV retrieval algorithm. A monthly climatology of aerosol layer height derived from observations by the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) sensor, and real-time AIRS (Atmospheric Infrared Sounder) CO observations are used in an upgraded version of the OMI near UV aerosol algorithm. AIRS CO measurements are used as a reliable tracer of carbonaceous aerosols, which allows the identification of smoke layers in areas and times of the year where the dust-smoke differentiation is difficult in the near-UV. The use of CO measurements also enables the identification of elevated levels of boundary layer pollution undetectable by near UV observations alone. In this paper we discuss the combined use of OMI, CALIOP and AIRS observations for the characterization of aerosol properties, and show a significant improvement in OMI aerosol retrieval capabilities.

  6. Hydrologic and climatologic data, 1965, Salt Lake County, Utah

    USGS Publications Warehouse

    Iorns, W.V.; Mower, Reed W.; Horr, C.A.

    1966-01-01

    An investigation of the water resources of Salt Lake County, Utah, was undertaken by the Water Resources Division of the U.S. Geological Survey in July 1963. This investigation is a cooperative project financed equally by the State of Utah and the Federal Government in accordance with an agreement between the State Engineer and the Geological Survey. The Utah Water and Power Board, Utah Fish and Game Commission, Salt Lake County Water Conservancy District, Metropolitan Water District of Salt Lake City, Salt Lake County, Kennecott Copper Corporation, Utah Power and Light Company, Salt Lake City Chamber of Commerce, and the Central Utah Water Conservancy District. contributed funds to the State Engineer's office toward support of the project.The investigation encompasses the collection and interpretation of a large variety of climatologic, hydrologic, and geologic data in and near Salt Lake County. Utah Basic-Data Release No. 11 contains data collected through 1964. This release contains climatologic and surface-water data for the 1965 water year (October 1964 to September 1965) and ground-water data collected during the 1965 calendar year. Similar annual releases will contain data collected during the remainder of the investigation, and interpretive reports will be prepared as the investigation proceeds. Organizations that furnished data are acknowledged in station descriptions and footnotes to tables.

  7. Hydrologic and climatologic data, 1966, Salt Lake County, Utah

    USGS Publications Warehouse

    Hely, A.G.; Mower, Reed W.; Horr, C.A.

    1967-01-01

    An investigation of the water resources of Salt Lake County, Utah, was undertaken by the Water Resources Division of the U.S. Geological Survey in July 1963. This investigation is a cooperative project financed equally by the State of Utah and the Federal Government in accordance with an agreement between the State Engineer and the Geological Survey. The Utah Water and Power Board, Utah Fish and Game Commission, Salt Lake County Water Conservancy District, Metropolitan Water District of Salt Lake City, Salt Lake County, Kennecott Copper Corporation, Utah Power and Light Company, Salt Lake City Chamber of Commerce, and the Central Utah Water Conservancy District contributed funds to the State Engineer's office toward support of the project.The investigation encompasses the collection and interpretation of a large variety of climatologic, hydrologic, and geologic data in and near Salt Lake County. Utah Basic-Data Releases 11 and 12 contain data collected through 1965. This release contains climatologic and surface-water data for the 1966 water year (October 1965 to September 1966) and groundwater data collected during the 1966 calendar year. Similar annual releases will contain data collected during the remainder of the investigation, and interpretive reports will be prepared as the investigation proceeds. Organizations that furnished data are acknowledged in station descriptions and footnotes to tables.

  8. MACv2-SP: a parameterization of anthropogenic aerosol optical properties and an associated Twomey effect for use in CMIP6

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Stevens, Bjorn; Fiedler, Stephanie; Kinne, Stefan

    A simple plume implementation of the second version (v2) of the Max Planck Institute Aerosol Climatology, MACv2-SP, is described. MACv2-SP provides a prescription of anthropogenic aerosol optical properties and an associated Twomey effect. It was created to provide a harmonized description of post-1850 anthropogenic aerosol radiative forcing for climate modeling studies. MACv2-SP has been designed to be easy to implement, change and use, and thereby enable studies exploring the climatic effects of different patterns of aerosol radiative forcing, including a Twomey effect. MACv2-SP is formulated in terms of nine spatial plumes associated with different major anthropogenic source regions. The shapemore » of the plumes is fit to the Max Planck Institute Aerosol Climatology, version 2, whose present-day (2005) distribution is anchored by surface-based observations. Two types of plumes are considered: one predominantly associated with biomass burning, the other with industrial emissions. These differ in the prescription of their annual cycle and in their optical properties, thereby implicitly accounting for different contributions of absorbing aerosol to the different plumes. A Twomey effect for each plume is prescribed as a change in the host model's background cloud-droplet population density using relationships derived from satellite data. Year-to-year variations in the amplitude of the plumes over the historical period (1850–2016) are derived by scaling the plumes with associated national emission sources of SO 2 and NH 3. Experiments using MACv2-SP are performed with the Max Planck Institute Earth System Model. The globally and annually averaged instantaneous and effective aerosol radiative forcings are estimated to be -0.6 and -0.5 W m -2, respectively. Forcing from aerosol–cloud interactions (the Twomey effect) offsets the reduction of clear-sky forcing by clouds, so that the net effect of clouds on the aerosol forcing is small; hence, the clear-sky forcing

  9. Source Attribution of Observed Absorption Profiles During the Two Column Aerosol Project (TCAP) Using a Regional Model

    NASA Astrophysics Data System (ADS)

    Fast, J. D.; Berg, L. K.; Chand, D.; Ferrare, R. A.; Flynn, C. J.; Hostetler, C. A.; Redemann, J.; Sedlacek, A. J., III; Shilling, J.; Shinozuka, Y.; Tomlinson, J. M.; Zelenyuk, A.

    2015-12-01

    Relatively large uncertainties remain in climate model predictions of absorption resulting from black carbon (BC) and brown carbon (BrC). In this study, we focus on comparing simulated profiles of BC, biomass burning aerosols, absorption, and other aerosol optical properties obtained from the regional WRF-Chem model with in situ and remote sensing measurements made during the Department of Energy's Two-Column Aerosol Project (TCAP). TCAP was designed to investigate changes in aerosol mixing state, aerosol radiative forcing, CCN concentration, and cloud-aerosol interactions in two atmospheric columns: one over Cape Cod, Massachusetts and another located approximately 200 km to the east over the ocean. Measurements from the NASA second-generation airborne High Resolution Spectral Lidar reveal the presence distinct aerosol layers associated with the marine boundary layer, residual layer transported over the ocean and in the free troposphere. Analyses of SP2 and aerosol optical measurements indicate that particles in the free troposphere were more 'aged' and had a lower single scattering albebo than for aerosol layers at lower altitudes; however, BC concentrations aloft were lower in the free troposphere. Instead, particle classes derived from the miniSPLAT single particle measurements suggest that the increased absorption aloft may be due biomass burning aerosols. The model suggests that ambient winds likely transported smoke from large wildfires in central Canada as well as smoke from other fires into the sampling domain. The simulated percentage of biomass burning aerosols was consistent with the miniSPLAT data, but the model currently treats all organic matter as non-absorbing. Therefore, we perform sensitivity simulations to examine how the model's absorption and AOD responds to assumptions used for BrC associated with biomass burning and whether the predicted profiles agree with absorption data and wavelength dependent AOD data from 4STAR.

  10. Climatic modification by CO2, H2O, and aerosol

    NASA Technical Reports Server (NTRS)

    Rasool, I.

    1972-01-01

    Research is reported on the effects of increasing the CO2, aerosols, and water content of the atmosphere on the surface temperature and climatology. An atmospheric model is described with the incoming solar radiation for a planetary albedo of 33 percent, surface temperature of 288 K, relative humidity of 75 percent, cloud cover of 48 percent, CO2 of 0.3 parts per thousand, and aerosol density of two million per square centimeter. The results show that if the CO2 increases by a factor of 1000 or more, the total pressure of the atmosphere increases, and the earth may become as hot as Venus. It is also shown that as the amount of dust particles in the atmosphere increases, the solar radiation decreases, and the surface temperature lowers.

  11. Ensembles of satellite aerosol retrievals based on three AATSR algorithms within aerosol_cci

    NASA Astrophysics Data System (ADS)

    Kosmale, Miriam; Popp, Thomas

    2016-04-01

    Ensemble techniques are widely used in the modelling community, combining different modelling results in order to reduce uncertainties. This approach could be also adapted to satellite measurements. Aerosol_cci is an ESA funded project, where most of the European aerosol retrieval groups work together. The different algorithms are homogenized as far as it makes sense, but remain essentially different. Datasets are compared with ground based measurements and between each other. Three AATSR algorithms (Swansea university aerosol retrieval, ADV aerosol retrieval by FMI and Oxford aerosol retrieval ORAC) provide within this project 17 year global aerosol records. Each of these algorithms provides also uncertainty information on pixel level. Within the presented work, an ensembles of the three AATSR algorithms is performed. The advantage over each single algorithm is the higher spatial coverage due to more measurement pixels per gridbox. A validation to ground based AERONET measurements shows still a good correlation of the ensemble, compared to the single algorithms. Annual mean maps show the global aerosol distribution, based on a combination of the three aerosol algorithms. In addition, pixel level uncertainties of each algorithm are used for weighting the contributions, in order to reduce the uncertainty of the ensemble. Results of different versions of the ensembles for aerosol optical depth will be presented and discussed. The results are validated against ground based AERONET measurements. A higher spatial coverage on daily basis allows better results in annual mean maps. The benefit of using pixel level uncertainties is analysed.

  12. Exploring reanalysis application for the purposes of climatological applications at regional scale

    NASA Astrophysics Data System (ADS)

    Kaspar, F.; Kaiser-Weiss, A.; Obregon, A.; Borsche, M.

    2014-12-01

    Recent advances in reanalysis methods yield new tools for climatological application. Here we use applications in Germany to discuss methodological issues at regional scale. Especially in the field of renewable energy planning and production there is a need for climatological information across all spatial scales, i.e., from climatology at a certain site to the spatial scale of national renewable energy production. Also, there is the need for the temporal resolution between the scales of a few minutes up to decadal changes. We explore the spatio-temporal scales where reanalyses can be used with benefit together with the traditional approaches which are based on station measurements only. Reanalyses can provide valuable additional information on larger scale variability, e.g. multi-annual variation over Germany. However, the change in the observing system, model errors and biases have to be carefully considered. On the other hand, the ground-based observation networks suffer from change of the station distribution, changes in instrumentation, measurements procedures and quality control as well as local changes which might modify their spatial representativity. All these effects might often been unknown or hard to characterize, although plenty of the meta-data information has been recorded for the German stations. European research activities on global and regional reanalysis are supported by the Framework Program 7 (FP7) of the European Commission as a preparation activity for the European COPERNICUS climate change service. Here we start from the user requirements for reanalyses as they were collected in the FP7 project CORE-CLIMAX. Second, we give an overview over the methods to determine whether a specific reanalysis is fit for a certain purpose (discussed in FP7 projects CORE-CLIMAX and UERRA) . Thirdly, we compare for an example application the feedback statistics from global (ERA-Interim) and regional (HErZ - COSMO) reanalyses and show which conclusion can be

  13. A global satellite-assisted precipitation climatology

    NASA Astrophysics Data System (ADS)

    Funk, C.; Verdin, A.; Michaelsen, J.; Peterson, P.; Pedreros, D.; Husak, G.

    2015-10-01

    Accurate representations of mean climate conditions, especially in areas of complex terrain, are an important part of environmental monitoring systems. As high-resolution satellite monitoring information accumulates with the passage of time, it can be increasingly useful in efforts to better characterize the earth's mean climatology. Current state-of-the-science products rely on complex and sometimes unreliable relationships between elevation and station-based precipitation records, which can result in poor performance in food and water insecure regions with sparse observation networks. These vulnerable areas (like Ethiopia, Afghanistan, or Haiti) are often the critical regions for humanitarian drought monitoring. Here, we show that long period of record geo-synchronous and polar-orbiting satellite observations provide a unique new resource for producing high-resolution (0.05°) global precipitation climatologies that perform reasonably well in data-sparse regions. Traditionally, global climatologies have been produced by combining station observations and physiographic predictors like latitude, longitude, elevation, and slope. While such approaches can work well, especially in areas with reasonably dense observation networks, the fundamental relationship between physiographic variables and the target climate variables can often be indirect and spatially complex. Infrared and microwave satellite observations, on the other hand, directly monitor the earth's energy emissions. These emissions often correspond physically with the location and intensity of precipitation. We show that these relationships provide a good basis for building global climatologies. We also introduce a new geospatial modeling approach based on moving window regressions and inverse distance weighting interpolation. This approach combines satellite fields, gridded physiographic indicators, and in situ climate normals. The resulting global 0.05° monthly precipitation climatology, the Climate

  14. Long-term Aerosol Lidar Measurements At CNR-IMAA

    NASA Astrophysics Data System (ADS)

    Mona, L.; Amodeo, A.; D'Amico, G.; Pandolfi, M.; Pappalardo, G.

    2006-12-01

    Actual estimations of the aerosol effect on the radiation budget are affected by a large uncertainties mainly due to the high inhomogeneity and variability of atmospheric aerosol, in terms of concentration, shape, size distribution, refractive index and vertical distribution. Long-term measurements of vertical profiles of aerosol optical properties are needed to reduce these uncertainties. At CNR-IMAA (40° 36'N, 15° 44' E, 760 m above sea level), a lidar system for aerosol study is operative since May 2000 in the framework of EARLINET (European Aerosol Research Lidar Network). Until August 2005, it provided independent measurements of aerosol extinction and backscatter at 355 nm and aerosol backscatter profiles at 532 nm. After an upgrade of the system, it provides independent measurements of aerosol extinction and backscatter profiles at 355 and 532 nm, and of aerosol backscatter profiles at 1064 nm and depolarization ratio at 532 nm. For these measurements, lidar ratio at 355 and 532 nm and Angstrom exponent profiles at 355/532 nm are also obtained. Starting on May 2000, systematic measurements are performed three times per week according to the EARLINET schedule and further measurements are performed in order to investigate particular events, like dust intrusions, volcanic eruptions and forest fires. A climatological study has been carried out in terms of the seasonal behavior of the PBL height and of the aerosol optical properties calculated inside the PBL itself. In the free troposphere, an high occurrences of Saharan dust intrusions (about 1 day of Saharan dust intrusion every 10 days) has been observed at CNR-IMAA because of the short distance from the Sahara region. During 6 years of observations, very peculiar cases of volcanic aerosol emitted by Etna volcano and aerosol released by large forest fires burning occurred in Alaska and Canada have been observed in the free troposphere at our site. Particular attention is devoted to lidar ratio both for the

  15. Critical analysis of documentary sources for Historical Climatology of Northern Portugal (17th-19th centuries)

    NASA Astrophysics Data System (ADS)

    Amorim, Inês; Sousa Silva, Luís; Garcia, João Carlos

    2017-04-01

    Critical analysis of documentary sources for Historical Climatology of Northern Portugal (17th-19th centuries) Inês Amorim CITCEM, Department of History, Political and International Studies, U. of Porto, Portugal. Luís Sousa Silva CITCEM, PhD Fellowship - FCT. João Carlos Garcia CIUHCT, Geography Department, U. of Porto, Portugal. The first major national project on Historical Climatology in Portugal, called "KLIMHIST: Reconstruction and model simulations of past climate in Portugal using documentary and early instrumental sources (17th-19th centuries)", ended in September 2015, coordinated by Maria João Alcoforado. This project began in March 2012 and counted on an interdisciplinary team of researchers from four Portuguese institutions (Centre of Geographical Studies, University of Trás-os-Montes and Alto Douro, University of Porto, and University of Évora), from different fields of knowledge (Geography, History, Biology, Climatology and Meteorology). The team networked and collaborated with other international research groups on Climate Change and Historical Climatology, resulting in several publications. This project aimed to reconstruct thermal and rainfall patterns in Portugal between the 17th and 19th centuries, as well as identify the main hydrometeorological extremes that occurred over that period. The basic methodology consisted in combining information from different types of anthropogenic sources (descriptive and instrumental) and natural sources (tree rings and geothermal holes), so as to develop climate change models of the past. The data collected were stored in a digital database, which can be searched by source, date, location and type of event. This database, which will be made publically available soon, contains about 3500 weather/climate-related records, which have begun to be studied, processed and published. Following this seminal project, other initiatives have taken place in Portugal in the area of Historical Climatology, namely a Ph

  16. Principles in Remote Sensing of Aerosol from MODIS Over Land and Ocean

    NASA Technical Reports Server (NTRS)

    Remer, L. A.; Kaufman, Y. J.; Tanre, D.; Chu, D. A.

    1999-01-01

    The well-calibrated spectral radiances measured by MODIS will be processed to retrieve daily aerosol properties that include optical thickness and mass loading over land and optical thickness, the mean particle size of the dominant mode and the ratio between aerosol modes over ocean. In addition, after launch, aerosol single scattering albedo will be calculated as an experimental product. The retrieval process over land is based on a dark target method that identifies appropriate targets in the mid-IR channels and uses an empirical relationship found between the mid-ER and the visible channels to estimate surface reflectance in the visible from the mid-HZ reflectance measured by satellite. The method employs new aerosol models for industrial, smoke and dust aerosol. The process for retrieving aerosol over the ocean makes use of the wide spectral band from 0.55-2.13 microns and a look-up table constructed from combinations of five accumulation modes and five coarse modes. Both the over land and over ocean algorithms have been validated with satellite and airborne radiance measurements. We estimate that MODIS will be able to measure aerosol optical thickness (t) to within 0.05 +/- 0.2t over land and to within 0.05 +/- 0.05t over ocean. Much of the earth's surface is located far from aerosol sources and experience very low aerosol optical thickness. Will the accuracy expected from MODIS retrievals be sufficient to measure the global aerosol direct and indirect forcing? We are attempting to answer this question using global model results and cloud climatology.

  17. Improving Aerosol and Visibility Forecasting Capabilities Using Current and Future Generations of Satellite Observations

    DTIC Science & Technology

    2012-09-30

    improving forecast performance over cloudy regions using the Ozone Monitoring Instrument (OMI) Aerosol Index; and 2) preparing for the post-MODIS...meteorological fields, the International Geosphere-Biosphere Programme (IGBP) SW and LW surface characteristics, and an ozone climatology are used as...The primary impact of CALIOP assimilation on the model is the redistribution of mass toward the boundary layer from the free troposphere . For high

  18. A climatology of polar stratospheric cloud composition between 2002 and 2012 based on MIPAS/Envisat observations

    NASA Astrophysics Data System (ADS)

    Spang, Reinhold; Hoffmann, Lars; Müller, Rolf; Grooß, Jens-Uwe; Tritscher, Ines; Höpfner, Michael; Pitts, Michael; Orr, Andrew; Riese, Martin

    2018-04-01

    The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument aboard the European Space Agency (ESA) Envisat satellite operated from July 2002 to April 2012. The infrared limb emission measurements provide a unique dataset of day and night observations of polar stratospheric clouds (PSCs) up to both poles. A recent classification method for PSC types in infrared (IR) limb spectra using spectral measurements in different atmospheric window regions has been applied to the complete mission period of MIPAS. The method uses a simple probabilistic classifier based on Bayes' theorem with a strong independence assumption on a combination of a well-established two-colour ratio method and multiple 2-D probability density functions of brightness temperature differences. The Bayesian classifier distinguishes between solid particles of ice, nitric acid trihydrate (NAT), and liquid droplets of supercooled ternary solution (STS), as well as mixed types. A climatology of MIPAS PSC occurrence and specific PSC classes has been compiled. Comparisons with results from the classification scheme of the spaceborne lidar Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on the Cloud-Aerosol-Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite show excellent correspondence in the spatial and temporal evolution for the area of PSC coverage (APSC) even for each PSC class. Probability density functions of the PSC temperature, retrieved for each class with respect to equilibrium temperature of ice and based on coincident temperatures from meteorological reanalyses, are in accordance with the microphysical knowledge of the formation processes with respect to temperature for all three PSC types.This paper represents unprecedented pole-covering day- and nighttime climatology of the PSC distributions and their composition of different particle types. The dataset allows analyses on the temporal and spatial development of the PSC formation process over

  19. Satellite-Based Assessment of Possible Dust Aerosols Semi-Direct Effect on Cloud Water Path over East Asia

    NASA Technical Reports Server (NTRS)

    Huang, Jianping; Lin, Bing; Minnis, Patrick; Wang, Tainhe; Wang, Xin; Hu, Yongxiang; Yi, Yuhong; Ayers, J. Kirk

    2006-01-01

    The semi-direct effects of dust aerosols are analyzed over eastern Asia using 2 years (June 2002 to June 2004) of data from the Clouds and the Earth s Radiant Energy System (CERES) scanning radiometer and MODerate Resolution Imaging Spectroradiometer (MODIS) on the Aqua satellite, and 18 years (1984 to 2001) of International Satellite Cloud Climatology Project (ISCCP) data. The results show that the water path of dust-contaminated clouds is considerably smaller than that of dust-free clouds. The mean ice water path (IWP) and liquid water path (LWP) of dusty clouds are less than their dust-free counterparts by 23.7% and 49.8%, respectively. The long-term statistical relationship derived from ISCCP also confirms that there is significant negative correlation between dust storm index and ISCCP cloud water path. These results suggest that dust aerosols warm clouds, increase the evaporation of cloud droplets and further reduce cloud water path, the so-called semi-direct effect. The semi-direct effect may play a role in cloud development over arid and semi-arid areas of East Asia and contribute to the reduction of precipitation.

  20. Global optical climatology of the free tropospheric aerosol from 1.0-micron satellite occultation measurements

    NASA Technical Reports Server (NTRS)

    Kent, G. S.; Schaffner, S. K.; Mccormick, M. P.

    1991-01-01

    Measurements of the aerosol/molecular extinction ratio at 1-micron wavelength, obtained from the SAGE I, SAGE II, and SAM II solar occultation satellite experiments between 1978 and 1986, have been used to study the global-scale behavior of the upper tropospheric aerosol. The distribution of extinction ratio values shows a pronounced mode between about 0.5 and 5 in all data subsets, regardless of latitude and season. Within a given latitude band and season with mode value is nearly constant over the altitude range from about 5 km above the earth's surface to 3 km below the tropopause. The mode shows a distinct seasonal variation, with maxima in local spring and summer, and is significantly enhanced following vlocanic injection of material into the stratosphere. South of latitude 20-deg N, mode values in the absence of volcanic contamination are normally between 0.5 and 1.0 north of 20-deg N, values up to about 5 are observed, probably associated with aerosol derived from surface dust or anthropogenic sources. A secondary mode, with extinction ratios of 30 or greater and little or no variation of extinction with wavelength, is apparent just below the tropopause. This mode is believed to be associated with thin cloud along the ray path from the sun to the satellite.

  1. Influence of Aerosols And Surface Reflectance On NO2 Retrieval Over China From 2005 to 2015

    NASA Astrophysics Data System (ADS)

    Liu, M.; Lin, J.

    2016-12-01

    Satellite observation is a powerful way to analysis annual and seasonal variations of nitrogen dioxide (NO2). However, much retrieval of vertical column densities (VCDs) of normally do not explicitly account for aerosol optical effects and surface reflectance anisotropy that vary with space and time. In traditional retrieval, aerosols' effects are often considered as cloud. However, China has complicated aerosols type and aerosol loading. Their optical properties may be very different from the cloud. Furthermore, China has undergone big changes in land use type in recent 10 years. Traditional climatology surface reflectance data may not have representation. In order to study spatial-temporal variation of and influences of these two factors on variations and trends, we use an improved retrieval method of VCDs over China, called the POMINO, based on measurements from the Ozone Monitoring Instrument (OMI), and we compare the results of without aerosol, without surface reflectance treatments and without both to the original POMINO product from 2005 to 2015. Furthermore, we will study correspondent spatial-temporal variations of aerosols, represented by MODIS aerosol optical depth (AOD) data and CALIOP extinction data; surface reflectance, represented by MODIS bidirectional reflectance distribution function (BRDF) data.

  2. Large-scale connection between aerosol optical depth and summer monsoon circulation, and precipitation over northeast Asia

    NASA Astrophysics Data System (ADS)

    Kim, Sang-Woo; Yoon, Soon-Chang; Choi, Suk-Jin; Choi, In-Jin

    2010-05-01

    We investigated the large-scale connection between columnar aerosol loads and summer monsoon circulation, and also the precipitation over northeast Asia using aerosol optical depth (AOD) data obtained from the 8-year MODIS, AERONET Sun/sky radiometer, and precipitation data acquired under the Global Precipitation Climatology Project (GPCP). These high-quality data revealed the large-scale link between AOD and summer monsoon circulation, precipitation in July over northeast Asian countries, and their distinct spatial and annual variabilities. Compared to the mean AOD for the entire period of 2001-2008, the increase of almost 40-50% in the AOD value in July 2005 and July 2007 was found over the downwind regions of China (Yellow Sea, Korean peninsula, and East Sea), with negative precipitation anomalies. This can be attributable to the strong westerly confluent flows, between cyclone flows by continental thermal low centered over the northern China and anti-cyclonic flows by the western North Pacific High, which transport anthropogenic pollution aerosols emitted from east China to aforementioned downwind high AOD regions along the rim of the Pacific marine airmass. In July 2002, however, the easterly flows transported anthropogenic aerosols from east China to the southwestern part of China in July 2002. As a result, the AOD off the coast of China was dramatically reduced in spite of decreasing rainfall. From the calculation of the cross-correlation coefficient between MODIS-derived AOD anomalies and GPCP precipitation anomalies over the period 2001-2008, we found negative correlations over the areas encompassed by 105-115E and 30-35N and by 120-140E and 35-40N (Yellow Sea, Korean peninsula, and East Sea). This suggests that aerosol loads over these regions are easily influenced by the Asian monsoon flow system and associated precipitation.

  3. The evaluation of a shuttle borne lidar experiment to measure the global distribution of aerosols and their effect on the atmospheric heat budget

    NASA Technical Reports Server (NTRS)

    Shipley, S. T.; Joseph, J. H.; Trauger, J. T.; Guetter, P. J.; Eloranta, E. W.; Lawler, J. E.; Wiscombe, W. J.; Odell, A. P.; Roesler, F. L.; Weinman, J. A.

    1975-01-01

    A shuttle-borne lidar system is described, which will provide basic data about aerosol distributions for developing climatological models. Topics discussed include: (1) present knowledge of the physical characteristics of desert aerosols and the absorption characteristics of atmospheric gas, (2) radiative heating computations, and (3) general circulation models. The characteristics of a shuttle-borne radar are presented along with some laboratory studies which identify schemes that permit the implementation of a high spectral resolution lidar system.

  4. SAM-CAAM: A Concept for Acquiring Systematic Aircraft Measurements to Characterize Aerosol Air Masses

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kahn, Ralph A.; Berkoff, Tim A.; Brock, Charles

    A modest operational program of systematic aircraft measurements can resolve key satellite aerosol data record limitations. Satellite observations provide frequent global aerosol amount maps but offer only loose aerosol property constraints needed for climate and air quality applications. In this paper, we define and illustrate the feasibility of flying an aircraft payload to measure key aerosol optical, microphysical, and chemical properties in situ. The flight program could characterize major aerosol airmass types statistically, at a level of detail unobtainable from space. It would 1) enhance satellite aerosol retrieval products with better climatology assumptions and 2) improve translation between satellite-retrieved opticalmore » properties and species-specific aerosol mass and size simulated in climate models to assess aerosol forcing, its anthropogenic components, and other environmental impacts. As such, Systematic Aircraft Measurements to Characterize Aerosol Air Masses (SAM-CAAM) could add value to data records representing several decades of aerosol observations from space; improve aerosol constraints on climate modeling; help interrelate remote sensing, in situ, and modeling aerosol-type definitions; and contribute to future satellite aerosol missions. Fifteen required variables are identified and four payload options of increasing ambition are defined to constrain these quantities. “Option C” could meet all the SAM-CAAM objectives with about 20 instruments, most of which have flown before, but never routinely several times per week, and never as a group. Aircraft integration and approaches to data handling, payload support, and logistical considerations for a long-term, operational mission are discussed. Finally, SAM-CAAM is feasible because, for most aerosol sources and specified seasons, particle properties tend to be repeatable, even if aerosol loading varies.« less

  5. SAM-CAAM: A Concept for Acquiring Systematic Aircraft Measurements to Characterize Aerosol Air Masses

    DOE PAGES

    Kahn, Ralph A.; Berkoff, Tim A.; Brock, Charles; ...

    2017-10-30

    A modest operational program of systematic aircraft measurements can resolve key satellite aerosol data record limitations. Satellite observations provide frequent global aerosol amount maps but offer only loose aerosol property constraints needed for climate and air quality applications. In this paper, we define and illustrate the feasibility of flying an aircraft payload to measure key aerosol optical, microphysical, and chemical properties in situ. The flight program could characterize major aerosol airmass types statistically, at a level of detail unobtainable from space. It would 1) enhance satellite aerosol retrieval products with better climatology assumptions and 2) improve translation between satellite-retrieved opticalmore » properties and species-specific aerosol mass and size simulated in climate models to assess aerosol forcing, its anthropogenic components, and other environmental impacts. As such, Systematic Aircraft Measurements to Characterize Aerosol Air Masses (SAM-CAAM) could add value to data records representing several decades of aerosol observations from space; improve aerosol constraints on climate modeling; help interrelate remote sensing, in situ, and modeling aerosol-type definitions; and contribute to future satellite aerosol missions. Fifteen required variables are identified and four payload options of increasing ambition are defined to constrain these quantities. “Option C” could meet all the SAM-CAAM objectives with about 20 instruments, most of which have flown before, but never routinely several times per week, and never as a group. Aircraft integration and approaches to data handling, payload support, and logistical considerations for a long-term, operational mission are discussed. Finally, SAM-CAAM is feasible because, for most aerosol sources and specified seasons, particle properties tend to be repeatable, even if aerosol loading varies.« less

  6. SAM-CAAM: A Concept for Acquiring Systematic Aircraft Measurements to Characterize Aerosol Air Masses.

    PubMed

    Kahn, Ralph A; Berkoff, Tim A; Brock, Charles; Chen, Gao; Ferrare, Richard A; Ghan, Steven; Hansico, Thomas F; Hegg, Dean A; Martins, J Vanderlei; McNaughton, Cameron S; Murphy, Daniel M; Ogren, John A; Penner, Joyce E; Pilewskie, Peter; Seinfeld, John H; Worsnop, Douglas R

    2017-10-01

    A modest operational program of systematic aircraft measurements can resolve key satellite-aerosol-data-record limitations. Satellite observations provide frequent, global aerosol-amount maps, but offer only loose aerosol property constraints needed for climate and air quality applications. We define and illustrate the feasibility of flying an aircraft payload to measure key aerosol optical, microphysical, and chemical properties in situ . The flight program could characterize major aerosol air-mass types statistically, at a level-of-detail unobtainable from space. It would: (1) enhance satellite aerosol retrieval products with better climatology assumptions, and (2) improve translation between satellite-retrieved optical properties and species-specific aerosol mass and size simulated in climate models to assess aerosol forcing, its anthropogenic components, and other environmental impacts. As such, Systematic Aircraft Measurements to Characterize Aerosol Air Masses (SAM-CAAM) could add value to data records representing several decades of aerosol observations from space, improve aerosol constraints on climate modeling , help interrelate remote-sensing, in situ, and modeling aerosol-type definitions , and contribute to future satellite aerosol missions. Fifteen Required Variables are identified, and four Payload Options of increasing ambition are defined, to constrain these quantities. "Option C" could meet all the SAM-CAAM objectives with about 20 instruments, most of which have flown before, but never routinely several times per week, and never as a group. Aircraft integration, and approaches to data handling, payload support, and logistical considerations for a long-term, operational mission are discussed. SAM-CAAM is feasible because, for most aerosol sources and specified seasons, particle properties tend to be repeatable , even if aerosol loading varies.

  7. The Deep South Clouds & Aerosols project: Improving the modelling of clouds in the Southern Ocean region

    NASA Astrophysics Data System (ADS)

    Morgenstern, Olaf; McDonald, Adrian; Harvey, Mike; Davies, Roger; Katurji, Marwan; Varma, Vidya; Williams, Jonny

    2016-04-01

    Southern-Hemisphere climate projections are subject to persistent climate model biases affecting the large majority of contemporary climate models, which degrade the reliability of these projections, particularly at the regional scale. Southern-Hemisphere specific problems include the fact that satellite-based observations comparisons with model output indicate that cloud occurrence above the Southern Ocean is substantially underestimated, with consequences for the radiation balance, sea surface temperatures, sea ice, and the position of storm tracks. The Southern-Ocean and Antarctic region is generally characterized by an acute paucity of surface-based and airborne observations, further complicating the situation. In recognition of this and other Southern-Hemisphere specific problems with climate modelling, the New Zealand Government has launched the Deep South National Science Challenge, whose purpose is to develop a new Earth System Model which reduces these very large radiative forcing problems associated with erroneous clouds. The plan is to conduct a campaign of targeted observations in the Southern Ocean region, leveraging off international measurement campaigns in this area, and using these and existing measurements of cloud and aerosol properties to improve the representation of clouds in the nascent New Zealand Earth System Model. Observations and model development will target aerosol physics and chemistry, particularly sulphate, sea salt, and non-sulphate organic aerosol, its interactions with clouds, and cloud microphysics. The hypothesis is that the cloud schemes in most GCMs are trained on Northern-Hemisphere data characterized by substantial anthropogenic or terrestrial aerosol-related influences which are almost completely absent in the Deep South.

  8. Tropical Atlantic Dust and Smoke Aerosol Variations Related to the Madden-Julian Oscillation in MODIS and MISR Observations

    NASA Technical Reports Server (NTRS)

    Guo, Yanjuan; Tian, Baijun; Kahn, Ralph A.; Kalashnikova, Olga; Wong, Sun; Waliser, Duane E.

    2013-01-01

    In this study, Moderate Resolution Imaging Spectroradiometer (MODIS) fine mode fraction and Multi-angle Imaging SpectroRadiometer (MISR) nonspherical fraction data are used to derive dust and smoke aerosol optical thickness (T(sub dust) and T(sub smoke)) over the tropical Atlantic in a complementary way: due to its wider swath, MODIS has 3-4 times greater sampling than MISR, but MISR dust discrimination is based on particle shape retrievals, whereas an empirical scheme is used for MODIS. MODIS and MISR show very similar dust and smoke winter climatologies. T(sub dust) is the dominant aerosol component over the tropical Atlantic, accounting for 40-70 percent of the total aerosol optical thickness (AOT), whereas T(sub smoke) is significantly smaller than T(sub dust). The consistency and high correlation between these climatologies and their daily variations lends confidence to their use for investigating the relative dust and smoke contributions to the total AOT variation associated with the Madden-Julian Oscillation (MJO). The temporal evolution and spatial patterns of the tdus anomalies associated with the MJO are consistent between MODIS and MISR: the magnitude of MJO-realted T(sub dust) anomalies is comparable to or even larger than that of the total T, while the T(sub smoke) anomaly represents about 15 percent compared to the total, which is quite different from their relative magnitudes to the total T on the climatological time scale. This suggests that dust and smoke are not influenced by the MJO in the same way. Based on correlation analysis, dust is strongly influenced by the MJO-modulated trade wind and precipitation anomalies, and can last as long as one MJO phase, whereas smoke is less affected.

  9. Hydrologic and climatologic data collected through 1964, Salt Lake County, Utah

    USGS Publications Warehouse

    Iorns, W.V.; Mower, Reed W.; Horr, C.A.

    1966-01-01

    An investigation of the water resources of Salt Lake County, Utah, was undertaken by the Water Resources Division of the U.S. Geological Survey in July 1963. This investigation is a cooperative project financed equally by the State of Utah and the Federal Government in accordance with an agreement between the State Engineer and the Geological Survey. The Utah Water and Power Board, Utah Fish and Game Commission, Salt Lake County Water Conservancy District, Metropolitan Water District of Salt Lake City, Salt Lake County, Kennecott Copper Corporation, Utah Power and Light Company, and Salt Lake City Chamber of Commerce contributed funds to the State Engineer's office toward support of the project.The investigation encompasses the collection and interpretation of a large variety of climatologic, hydrologic, and geologic data in and near Salt Lake County. This basic-data report sets forth climatologic and surface-water data collected by project personnel and others during the water year beginning October 1, 1963, and ending September 30, 1964, and ground-water data collected by project personnel and others for the period July 1, 1963, through December 31, 1964. Included also are some earlier ground-water data not previously published. Organizations that furnished data are acknowledged in station descriptions and footnotes to tables. Data collected during the period of investigation will be published in annual basic-data releases and an interpretative report will be published at the completion of the investigation.

  10. Seasonal Characteristics of Tropical Ozone Profiles using the SHADOZ Ozonesonde Data Set: Comparisons with TOMS Tropical Ozone Climatology

    NASA Technical Reports Server (NTRS)

    Witte, J. C.; Thompson, A. M.; Bhartia, P. K. (Technical Monitor)

    2002-01-01

    Advances in tropospheric ozone data products being developed for tropical and subtropical regions using TOMS (Total Ozone Mapping Spectrometer) and other satellites are motivating efforts to renew and expand the collection of balloon-borne ozonesonde observations. The SHADOZ (Southern Hemisphere ADditional OZonesondes) project is a web-based archive established since 1998. It's goals are to support validation of TOMS and SBUV (Solar Backscatter UV) satellite ozone measurements and to improve remote sensing techniques for estimating tropical and subtropical ozone. Profile data are taken from balloon-borne ozonesondes, currently at 11 stations coordinating weekly to bi-weekly launches. Station data are publically available at a central location via the internet: . Since the start of the project, the SHADOZ archive has accumulated over 1500 ozonesonde profiles. Data also includes measurements from various SHADOZ supported field campaigns, such as, the Indian Ocean Experiment (INDOEX), Sounding of Ozone and Water in the Equatorial Region (SOWER) and Aerosols99 Atlantic Cruise. Using data from the archive, profile climatologies from selected stations will be shown to 1/characterize the variability of tropospheric tropical ozone among stations, 2/illustrate the seasonal offsets with respect to the tropical profile used in the TOMS v7 algorithm, and 3/estimate the potential error in TOMS retrieval estimates of the tropospheric portion of the atmosphere.

  11. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Richard A. Ferrare; David D. Turner

    Project goals: (1) Use the routine surface and airborne measurements at the ARM SGP site, and the routine surface measurements at the NSA site, to continue our evaluations of model aerosol simulations; (2) Determine the degree to which the Raman lidar measurements of water vapor and aerosol scattering and extinction can be used to remotely characterize the aerosol humidification factor; (3) Use the high temporal resolution CARL data to examine how aerosol properties vary near clouds; and (4) Use the high temporal resolution CARL and Atmospheric Emitted Radiance Interferometer (AERI) data to quantify entrainment in optically thin continental cumulus clouds.

  12. Using MODIS Cloud Regimes to Sort Diagnostic Signals of Aerosol-Cloud-Precipitation Interactions

    PubMed Central

    Oreopoulos, Lazaros; Cho, Nayeong; Lee, Dongmin

    2018-01-01

    Coincident multi-year measurements of aerosol, cloud, precipitation and radiation at near-global scales are analyzed to diagnose their apparent relationships as suggestive of interactions previously proposed based on theoretical, observational, and model constructs. Specifically, we examine whether differences in aerosol loading in separate observations go along with consistently different precipitation, cloud properties, and cloud radiative effects. Our analysis uses a cloud regime (CR) framework to dissect and sort the results. The CRs come from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor and are defined as distinct groups of cloud systems with similar co-variations of cloud top pressure and cloud optical thickness. Aerosol optical depth used as proxy for aerosol loading comes from two sources, MODIS observations, and the MERRA-2 re-analysis, and its variability is defined with respect to local seasonal climatologies. The choice of aerosol dataset impacts our results substantially. We also find that the responses of the marine and continental component of a CR are frequently quite disparate. Overall, CRs dominated by warm clouds tend to exhibit less ambiguous signals, but also have more uncertainty with regard to precipitation changes. Finally, we find weak, but occasionally systematic co-variations of select meteorological indicators and aerosol, which serves as a sober reminder that ascribing changes in cloud and cloud-affected variables solely to aerosol variations is precarious. PMID:29651373

  13. Using MODIS Cloud Regimes to Sort Diagnostic Signals of Aerosol-Cloud-Precipitation Interactions.

    PubMed

    Oreopoulos, Lazaros; Cho, Nayeong; Lee, Dongmin

    2017-05-27

    Coincident multi-year measurements of aerosol, cloud, precipitation and radiation at near-global scales are analyzed to diagnose their apparent relationships as suggestive of interactions previously proposed based on theoretical, observational, and model constructs. Specifically, we examine whether differences in aerosol loading in separate observations go along with consistently different precipitation, cloud properties, and cloud radiative effects. Our analysis uses a cloud regime (CR) framework to dissect and sort the results. The CRs come from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor and are defined as distinct groups of cloud systems with similar co-variations of cloud top pressure and cloud optical thickness. Aerosol optical depth used as proxy for aerosol loading comes from two sources, MODIS observations, and the MERRA-2 re-analysis, and its variability is defined with respect to local seasonal climatologies. The choice of aerosol dataset impacts our results substantially. We also find that the responses of the marine and continental component of a CR are frequently quite disparate. Overall, CRs dominated by warm clouds tend to exhibit less ambiguous signals, but also have more uncertainty with regard to precipitation changes. Finally, we find weak, but occasionally systematic co-variations of select meteorological indicators and aerosol, which serves as a sober reminder that ascribing changes in cloud and cloud-affected variables solely to aerosol variations is precarious.

  14. Characterization of the 3D distribution of ozone and coarse aerosols in the Troposphere using IASI thermal infrared satellite observations

    NASA Astrophysics Data System (ADS)

    Cuesta, J.; Eremenko, M.; Dufour, G.; Hoepfner, M.; Orphal, J.

    2012-04-01

    ., 2006 ACP]. As a priori inputs, we consider climatological ozone profiles, ECMWF meteorological fields and aerosol refractive index and size distributions based on desert dust [Hess et al., 1998 AMS] and smoke [Tsay and Stephens 1990] climatologies. We have used our joint ozone/aerosol retrieval to analyse two major events: i) the Russian fires during the heatwave of summer 2010 in the Moscow area and ii) a desert dust outbreak reaching Beijing in springtime 2008. We propose to present our results on these two study cases, as well as the performance assessment of our technique.

  15. Effects of the Urban Heat Island on Aerosol pH

    NASA Astrophysics Data System (ADS)

    Battaglia, M., Jr.; Douglas, S.; Hennigan, C. J.

    2017-12-01

    The urban heat island (UHI) is a widely observed phenomenon whereby urban environments have higher temperature (T) and lower relative humidity (RH) than surrounding suburban and rural areas. Both of these factors affect the partitioning of semi-volatile species found in the atmosphere, such as nitric acid and ammonia. These species are inherently tied to aerosol pH, which is a key parameter driving some atmospheric chemical processes and environmental effects of aerosols. In this study, we characterized the effect of the UHI on aerosol pH in Baltimore, MD and Chicago, IL. These cities were selected based on differences in climatology, source influences, and atmospheric composition. Meteorological and atmospheric composition data from the urban centers and surrounding rural locations were used as inputs to the ISORROPIA-II aerosol thermodynamic model to compute gas/particle partitioning, aerosol liquid water content, and aerosol pH. Dramatic differences in aerosol liquid water (ALW) content were found in both cities and were attributable to the T and RH differences (UHI effect). The urban-rural differences in ALW result in urban aerosol pH that is systematically lower (more acidic) than rural aerosol pH for identical atmospheric composition. The UHI in Baltimore is most intense during the summer and at night, with differences of up to 1 pH unit predicted during these times. Similarly, the UHI in Chicago is most intense during the summer and at night; however, the atmospheric composition in Chicago shows a mediating effect, with differences of up to 0.65 pH units predicted during these times. These results are likely to have broad implications for chemistry occurring in and around urban atmospheres globally, although the magnitude of the effect may differ based on the UHI characteristic of each urban environment.

  16. Aerosol Microphysics and Radiation Integration

    DTIC Science & Technology

    2007-09-30

    http://www.nrlmry.navy.mil/ flambe / LONG-TERM GOALS This project works toward the development and support of real time global prognostic aerosol...Burning Emissions ( FLAMBE ) project were transition to the Fleet Numerical Oceanographic Center (FNMOC) Monterey in FY07. Meteorological guidance...Hyer, E. J. and J. S. Reid (2006), Evaluating the impact of improvements to the FLAMBE smoke source model on forecasts of aerosol distribution

  17. Recent increase in aerosol loading over the Australian arid zone

    NASA Astrophysics Data System (ADS)

    Mitchell, R. M.; Campbell, S. K.; Qin, Y.

    2009-10-01

    Collocated sun photometer and nephelometer measurements at Tinga Tingana in the Australian Outback over the decade 1997-2007 show a significant increase in aerosol loading following the onset of severe drought conditions in 2002. The mean mid-visible scattering coefficient obtained from nephelometer measurements over the period 2003-2007 is approximately double that recorded over the preceding 5 yr, with consistent trends in the column aerosol optical depth derived from the sun photometer. This increase is confined to the season of dust activity, particularly September to March. In contrast, background aerosol levels during May, June and July remained stable. The enhanced aerosol loadings during the latter 5 yr of the study period can be understood as a combination of dune destabilisation through loss of ephemeral vegetation and surface crust, and the changing supply of fluvial sediments to ephemeral lakes and floodplains within the Lake Eyre Basin. Major dust outbreaks are generally highly localised, although significant dust activity was observed at Tinga Tingana on 50% of days when a major event occurred elsewhere in the Lake Eyre Basin, suggesting frequent basin-wide dust mobilisation. Combined analysis of aerosol optical depth and scattering coefficient shows weak correlation between the surface and column aerosol (R2=0.24). The aerosol scale height is broadly distributed with a mode typically between 2-3 km, with clearly defined seasonal variation. Climatological analysis reveals bimodal structure in the annual cycle of aerosol optical depth, with a summer peak related to maximal dust activity, and a spring peak related to lofted fine-mode aerosol. There is evidence for an increase in near-surface aerosol during the period 2003-2007 relative to 1997-2002, consistent with an increase in dust activity. This accords with an independent finding of increasing aerosol loading over the Australian region as a whole, suggesting that rising dust activity over the Lake

  18. Aerosol Radiative Forcing over North India during Pre-Monsoon Season using WRF-Chem

    NASA Astrophysics Data System (ADS)

    Misra, A.; Kumar, K.; Michael, M.; Tripathi, S. N.

    2013-12-01

    Study of aerosols is important for a fair understanding of the Earth climate system. This requires knowledge of the physical, chemical, optical, and morphological properties of aerosols. Aerosol radiative forcing provides information on the effect of aerosols on the Earth radiation budget. Radiative forcing estimates using model data provide an opportunity to examine the contribution of individual aerosol species to overall radiative forcing. We have used Weather Research and Forecast with Online Chemistry (WRF-Chem) derived aerosol concentration data to compute aerosol radiative forcing over north India during pre-monsoon season of 2008, 2009, and 2010. WRF-Chem derived mass concentrations are converted to number concentrations using standard procedure. Optical Properties of Aerosol and Cloud (OPAC) software package is used to compute extinction and scattering coefficients, and asymmetry parameter. Computations are performed at different altitudes and the obtained values are integrated to get the column optical properties. Santa Barbara Discrete Ordinate Radiative Transfer (SBDART) model is used to calculate the radiative forcing at surface and top-of-atmosphere. Higher values of aerosol radiative forcing are observed over desert region in western Indian state of Rajasthan, and Punjab of Pakistan. Contribution of individual aerosol species to atmospheric radiative forcing is also assessed. Dust radiative forcing is high over western India. Radiative forcing due to BC and water-soluble (WASO) aerosols are higher over north-west Indian states of Punjab and Haryana, and the Indo-Gangetic Basin. A pool of high WASO optical depth and radiative forcing is observed over the Indo-Bangladesh border. The findings of aerosol optical depth and radiative forcing are consistent with the geography and prevailing aerosol climatology of various regions. Heating rate profiles due to total aerosols and only due to BC have been evaluated at selected stations in north India. They show

  19. Validation of Global Climatologies of Trace Gases Using NASA Global Tropospheric Experiment (GTE) Data

    NASA Technical Reports Server (NTRS)

    Courchaine, Brian; Venable, Jessica C.

    1995-01-01

    Methane is an important trace gas because it is a greenhouse gas that affects the oxidative capacity of the atmosphere. It is produced from biological and anthropogenic sources, and is increasing globally at a rate of approximately 0.6% per year [Climate Change 1992, IPCC]. By using National Oceanic and Atmospheric Administration/Climate Monitoring and Diagnostics Laboratory (NOAA/CMDL) ground station data, a global climatology of methane values was produced. Unfortunately, because the NOAA/CMDL ground stations are so sparse, the global climatology is low resolution. In order to compensate for this low resolution data, it was compared to in-situ flight data obtained from the NASA Global Tropospheric Experiment (GTE). The smoothed ground station data correlated well with the flight data. Thus, for the first time it is shown that the smoothing process used to make global contours of methane using the ground stations is a plausible way to approximate global atmospheric concentrations of the gas. These verified climatologies can be used for testing large-scale models of chemical production, destruction, and transport. This project develops the groundwork for further research in building global climatologies from sparse ground station data and studying the transport and distribution of trace gases.

  20. Theoretical Characterization of the Radiative Properties of Dust Aerosol for the Air Force Combat Climatology Center Point Analysis Intelligence System

    DTIC Science & Technology

    2007-03-01

    dust aerosol is known to absorb radiation in these wavelengths. Therefore, the absorptive properties of the aerosol must be taken into account to...of the dust aerosol on radiation propagation is complicated. The study addressed this problem by modeling various radiative transfer situations...are ubiquitous in nature and frequently are the determining factor in the amount of radiation received at a sensor.” The horizontal and vertical

  1. Synchronised Aerosol Mass Spectrometer Measurements across Europe

    NASA Astrophysics Data System (ADS)

    Nemitz, Eiko

    2010-05-01

    Up to twelve Aerodyne Aerosol Mass Spectrometers (AMSs) were operated simultaneously at rural and background stations (EMEP and EUSAAR sites) across Europe. Measurements took place during three intensive periods, in collaboration between the European EUCAARI IP and the EMEP monitoring activities under the UNECE Convention for Long-Range Transboundary Air Pollution (CLRTAP) during three contrasting months (May 2008, Sep/Oct 2008, Feb/Mar 2009). These measurements were conducted, analysed and quality controlled carefully using a unified protocol, providing the largest spatial database of aerosol chemical composition measured with a unified online technique to date, and a unique snapshots of the European non-refractory submicron aerosol climatology. As campaign averages over all active monitoring sites, organics represent 28 to 43%, sulphate 18 to 25%, ammonium 13 to 15% and nitrate 15 to 36% of the resolved aerosol mass, with the highest relative nitrate contribution during the Feb/Mar campaign. The measurements demonstrate that in NW Europe (e.g. Ireland, UK, The Netherlands, Germany, Switzerland) the regional submicron aerosol tends to be neutralised and here nitrates make a major contribution to the aerosol mass. By contrast, periods with low nitrate and acidic aerosol were observed at sites in S and E Europe (e.g. Greece, Finland), presumably due to a combination of larger SO2 point sources in Easter Europe, smaller local NH3 sources and, in the case of Greece, higher temperatures. While at the more marine and remote sites (Ireland, Scotland, Finland) nitrate concentrations were dominated by episodic transport phenomena, at continental sites (Switzerland, Germany, Hungary) nitrate followed a clear diurnal cycle, reflecting the thermodynamic behaviour of ammonium nitrate. The datasets clearly shows spatially co-ordinated, large-scale pollution episodes of organics, sulphate and nitrate, the latter being most pronounced during the Feb/Mar campaign. At selected

  2. Multispectral information for gas and aerosol retrieval from TANSO-FTS instrument

    NASA Astrophysics Data System (ADS)

    Herbin, H.; Labonnote, L. C.; Dubuisson, P.

    2012-11-01

    The Greenhouse gases Observing SATellite (GOSAT) mission and in particular TANSO-FTS instrument has the advantage to measure simultaneously the same field of view in different spectral ranges with a high spectral resolution. These features are promising to improve, not only, gaseous retrieval in clear sky or scattering atmosphere, but also to retrieve aerosol parameters. Therefore, this paper is dedicated to an Information Content (IC) analysis of potential synergy between thermal infrared, shortwave infrared and visible, in order to obtain a more accurate retrieval of gas and aerosol. The latter is based on Shannon theory and used a sophisticated radiative transfer algorithm developed at "Laboratoire d'Optique Atmosphérique", dealing with multiple scattering. This forward model can be relied to an optimal estimation method, which allows simultaneously retrieving gases profiles and aerosol granulometry and concentration. The analysis of the information provided by the spectral synergy is based on climatology of dust, volcanic ash and biomass burning aerosols. This work was conducted in order to develop a powerful tool that allows retrieving simultaneously not only the gas concentrations but also the aerosol characteristics by selecting the so called "best channels", i.e. the channels that bring most of the information concerning gas and aerosol. The methodology developed in this paper could also be used to define the specifications of future high spectral resolution mission to reach a given accuracy on retrieved parameters.

  3. Giant aerosol observations with cloud radar: methodology and effects

    NASA Astrophysics Data System (ADS)

    Guma Claramunt, Pilar; Madonna, Fabio; Amodeo, Aldo; Bauer-Pfundstein, Matthias; Papagiannopoulos, Nikolaos; Pappalardo, Gelsomina

    2017-04-01

    Giant aerosol particles can act as Giant Cloud Condensation Nuclei (GCCN), and determine the droplet concentration at the cloud formation, the clouds albedo and lifetime, and the precipitation formation. In addition, depending on their composition, they can also act as IN. It is not yet clear if they can also expedite rain processes. The main techniques used nowadays in measuring aerosols, which are lidar and sun photometer, cannot retrieve aerosol microphysical properties for particles bigger than a few microns, which means that they do not account for giant aerosols. Therefore, the distribution and impact in the atmosphere and climate of these particles is not well known and the aerosol transport models largely underestimate them. Recent studies have demonstrated that cloud radars are able to detect ultragiant volcanic aerosols also at a large distance from the source. In this study, an innovative methodology for the observation of giant aerosols using the millimeter wavelength radar has been developed and applied to 6 years of measurements carried out at CNR-IMAA Atmospheric Observatory (CIAO), in Potenza, South Italy, finding more than 40 giant aerosol events per year and a good agreement with the aerosol climatologic data. Besides, the effects of giant aerosols in the local and regional meteorology have been studied by correlating several atmospheric variables in the time period following the observation of giant particles. The meteorological situation has been assessed through the data classification into cases characterized by different pressure vertical velocities at the upper atmosphere (400 hPa), Giant aerosols are correlated to lower values of the Cloud Optical Depth (COD) in presence of stable or unstable atmospheric conditions while higher values are found for an intermediate stability. The giant aerosols effects on the Liquid Water Path (LWP) are closely linked to those in the Aerosol Optical Thickness (AOD). The highest increases in the LWP occurs

  4. Observational and Dynamical Wave Climatologies. VOS vs Satellite Data

    NASA Astrophysics Data System (ADS)

    Grigorieva, Victoria; Badulin, Sergei; Chernyshova, Anna

    2013-04-01

    The understanding physics of wind-driven waves is crucially important for fundamental science and practical applications. This is why experimental efforts are targeted at both getting reliable information on sea state and elaborating effective tools of the sea wave forecasting. The global Visual Wave Observations and satellite data from the GLOBWAVE project of the European Space Agency are analyzed in the context of these two viewpoints. Within the first "observational" aspect we re-analyze conventional climatologies of all basic wave parameters for the last decades [5]. An alternative "dynamical" climatology is introduced as a tool of prediction of dynamical features of sea waves on global scales. The features of wave dynamics are studied in terms of one-parametric dependencies of wave heights on wave periods following the theoretical concept of self-similar wind-driven seas [3, 1, 4] and recently proposed approach to analysis of Voluntary Observing Ship (VOS) data [2]. Traditional "observational" climatologies based on VOS and satellite data collections demonstrate extremely consistent pictures for significant wave heights and dominant periods. On the other hand, collocated satellite and VOS data show significant differences in wave heights, wind speeds and, especially, in wave periods. Uncertainties of visual wave observations can explain these differences only partially. We see the key reason of this inconsistency in the methods of satellite data processing which are based on formal application of data interpolation methods rather than on up-to-date physics of wind-driven waves. The problem is considered within the alternative climatology approach where dynamical criteria of wave height-to-period linkage are used for retrieving wave periods and constructing physically consistent dynamical climatology. The key dynamical parameter - exponent R of one-parametric dependence Hs ~ TR shows dramatically less pronounced latitudinal dependence as compared to observed Hs

  5. Seasonal evolution of the West African heat low: a climatological perspective

    NASA Astrophysics Data System (ADS)

    Lavaysse, C.; Flamant, C.; Janicot, S.; Parker, D. J.; Lafore, J.-P.; Sultan, B.; Pelon, J.

    2009-08-01

    year 2006 (the year of the African Monsoon Multidisciplinary Analysis project Special Observation Period) is analysed and compared with the climatological results. The operational ECMWF analyses were used for that purpose. Except in April, the spatial distribution of the WAHL remains relatively unchanged and agrees with the climatology. The onset of the SHL in 2006 occurs on 18 June, which is close to the climatological date, in spite of the delay in the onset of the rainy season in Sahel.

  6. The Adaptive Ecosystem Climatology (AEC): Design and Development

    NASA Astrophysics Data System (ADS)

    deRada, S.; Penta, B.; McCarthy, S.; Gould, R. W., Jr.

    2016-02-01

    The concept of ecosystem-based management (EBM), recently introduced to rectify the shortcomings of single-species management policies, has been widely accepted as a basis for the conservation and management of natural resources. In line with NOAA's Integrated Ecosystem Assessment (IEA) Program, EBM is an integrated approach that considers the entire ecosystem and the interactions among species rather than focusing on individual components. This integrative approach relies on heterogeneous data, physical as well as biogeochemical data, among many others. Relative to physical data, however, marine biogeochemical records, also critical in IEA and EBM, are still lacking, both in terms of mature models and in terms of observational data availability. TheAdaptive Ecosystem Climatology (AEC) was conceived as a novel approach to address these limitations, mitigating the shortcomings of the individual components and combining their strengths to enhance decision-making activities. AEC is designed on the concept that a high-frequency climatology can be used as a baseline into which available observational data can be ingested to produce a higher accuracy product. In the absence of observations, the climatology acts as a best estimate. AEC was developed using a long-term simulation of a coupled biophysical numerical model configured for the Gulf of Mexico. Using the model results, we constructed a three-dimensional, dynamically balanced, gridded, static climatology for each calendar day. Using this `static' climatology as a background `first guess', observations from a particular date are ingested via optimal interpolation to `nudge' the climatology toward current conditions, thus providing representative fields for that date (adaptive climatology). With this adaptive approach, AEC can support a variety of EBM objectives, from fisheries, to resource management, to coastal resilience.

  7. Mars Geoscience Climatology Orbiter (MGCO) extended study: Technical volume

    NASA Technical Reports Server (NTRS)

    1983-01-01

    The FLTSATCOM Earth orbiting communications satellite is a prominent candidate to serve as the Mars Geoscience Climatology Orbiter (MGCO) spacecraft. Major aspects directly applicable are: (1) the incorporation of solid orbit insertion motor; (2) the ability to cruise to Mars in the spin-stabilized mode; (3) ample capability for payload mass and power; (4) attitude control tried to nadir and orbit plane coordinates; (5) exemplary Earth orbital performance record and projected lifetime; and (6) existence of an on-going procurement into the MGCO time period.

  8. A Global, Decadal, Quantitative Record of Absorbing Aerosols above Cloud Using OMI's Near-UV Observations

    NASA Astrophysics Data System (ADS)

    Torres, O.; Jethva, H. T.; Ahn, C.

    2016-12-01

    Aerosol-cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of an adequate knowledge of the complex microphysical and radiative processes of the aerosol-cloud system. The situations when aerosols and clouds are found in the same atmospheric column, for instance, when light-absorbing aerosols such as biomass burning generated carbonaceous particles or wind-blown dust overlay low-level cloud decks, are commonly found over several regions of the world. Contrary to the known cooling effects of these aerosols in cloud-free scenario over dark surface, the overlapping situation of absorbing aerosols over cloud can potentially exert a significant level of atmospheric absorption and produces a positive radiative forcing (warming) at top-of-atmosphere. The magnitude of direct radiative effects of aerosols above cloud directly depends on the aerosol loading, microphysical and optical properties of the aerosol layer and the underlying cloud deck, and geometric cloud fraction. We help in addressing this problem by introducing a novel product of above-cloud aerosol optical depth (ACAOD) of absorbing aerosols retrieved from near-UV observations made by the Ozone Monitoring Instrument (OMI) on board NASA's Aura platform. Physically based on the strong `color ratio' effect in the near-UV caused by the spectral absorption of aerosols above cloud, the algorithm, formally named as OMACA, retrieves the optical depths of aerosols and clouds simultaneously under a prescribed state of atmosphere. Here, we present the algorithm architecture and results from an 11-year global record (2005-2015) including global climatology of frequency of occurrence and ACAOD. The theoretical uncertainty analysis and planned validation activities using measurements from upcoming field campaigns are also discussed.

  9. Characterization of urban aerosol using aerosol mass spectrometry and proton nuclear magnetic resonance spectroscopy

    NASA Astrophysics Data System (ADS)

    Cleveland, M. J.; Ziemba, L. D.; Griffin, R. J.; Dibb, J. E.; Anderson, C. H.; Lefer, B.; Rappenglück, B.

    2012-07-01

    Particulate matter was measured during August and September of 2006 in Houston as part of the Texas Air Quality Study II Radical and Aerosol Measurement Project. Aerosol size and composition were determined using an Aerodyne quadrupole aerosol mass spectrometer. Aerosol was dominated by sulfate (4.1 ± 2.6 μg m-3) and organic material (5.5 ± 4.0 μg m-3), with contributions of organic material from both primary (˜32%) and secondary (˜68%) sources. Secondary organic aerosol appears to be formed locally. In addition, 29 aerosol filter samples were analyzed using proton nuclear magnetic resonance (1H NMR) spectroscopy to determine relative concentrations of organic functional groups. Houston aerosols are less oxidized than those observed elsewhere, with smaller relative contributions of carbon-oxygen double bonds. These particles do not fit 1H NMR source apportionment fingerprints for identification of secondary, marine, and biomass burning organic aerosol, suggesting that a new fingerprint for highly urbanized and industrially influenced locations be established.

  10. Comparative Climatology of Terrestrial Planets

    NASA Astrophysics Data System (ADS)

    Mackwell, Stephen J.; Simon-Miller, Amy A.; Harder, Jerald W.; Bullock, Mark A.

    stimulate further research on this critical subject. The study of climate involves much more than understanding atmospheric processes. This subtlety is particularly appreciated for Earth, where chemical cycles, geology, ocean influences, and biology are considered in most climate models. In Part IV, Surface and Interior, we look at the role that geochemical cycles, volcanism, and interior mantle processes play in the stability and evolution of terrestrial planetary climates. There is one vital commonality between the climates of all the planets of the solar system: Regardless of the different processes that dominate each of the climates of Earth, Mars, Venus, and Titan, they are all ultimately forced by radiation from the same star, albeit at variable distances. In Part V, Solar Influences, we discuss how the Sun's early evolution affected the climates of the terrestrial planets, and how it continues to control the temperatures and compositions of planetary atmospheres. This will be of particular interest as models of exoplanets, and the influences of much different stellar types and distances, are advanced by further observations. Comparisons of atmospheric and climate processes between the planets in our solar system has been a focus of numerous conferences over the past decade, including the Exoclimes conference series. In particular, this book project was closely tied to a conference on Comparative Climatology of Terrestrial Planets that was held in Boulder, Colorado, on June 25-28, 2012. This book benefited from the opportunity for the author teams to interact and obtain feedback from the broader community, but the chapters do not in general tie directly to presentations at the conference. The conference, which was organized by a diverse group of atmospheric and climate scientists led by Mark Bullock and Lori Glaze, sought to build connections between the various communities, focusing on synergies and complementary capabilities. Discussion panels at the end of most

  11. A Long-term Record of Saharan Dust Aerosol Properties from TOMS Observations: Optical Depth and Single Scattering Albedo

    NASA Technical Reports Server (NTRS)

    Torres, Omar; Bhartia, P. K.; Herman, J. R.; Einaudi, Franco (Technical Monitor)

    2000-01-01

    The interaction between the strong Rayleigh scattering in the near UV spectral region (330-380 nm) and the processes of aerosol absorption and scattering, produce a clear spectral signal in the upwelling radiance at the top of the atmosphere. This interaction is the basis of the TOMS (Total Ozone Mapping Spectrometer) aerosol retrieval technique that can be used for their characterization and to differentiate non-absorbing sulfates from strongly UV-absorbing aerosols such as mineral dust. For absorbing aerosols, the characterization is in terms of the optical depth and single scattering albedo with assumptions about the aerosol plume height. The results for non-absorbing aerosols are not dependent on plume height. Although iron compounds represent only between 5% to 8% of desert dust aerosol mass, hematite (Fe2O3) accounts for most of the near UV absorption. Because of the large ultraviolet absorption characteristic of hematite, the near UV method of aerosol sensing is especially suited for the detection and characterization of desert dust aerosols. Using the combined record of near UV measurements by the Nimbus7 (1978-1992) and Earth Probe (1996-present) TOMS instruments, a global longterm climatology of near UV optical depth and single scattering albedo has been produced. The multi-year long record of mineral aerosol properties over the area of influence of the Saharan desert, will be discussed.

  12. Simulating Aerosol Indirect Effects with Improved Aerosol-Cloud- Precipitation Representations in a Coupled Regional Climate Model

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Zhang, Yang; Leung, L. Ruby; Fan, Jiwen

    This is a collaborative project among North Carolina State University, Pacific Northwest National Laboratory, and Scripps Institution of Oceanography, University of California at San Diego to address the critical need for an accurate representation of aerosol indirect effect in climate and Earth system models. In this project, we propose to develop and improve parameterizations of aerosol-cloud-precipitation feedbacks in climate models and apply them to study the effect of aerosols and clouds on radiation and hydrologic cycle. Our overall objective is to develop, improve, and evaluate parameterizations to enable more accurate simulations of these feedbacks in high resolution regional and globalmore » climate models.« less

  13. Tropical Atlantic Dust and Smoke Aerosol Variabilities Related to the Madden-Julian Oscillation in MODIS and MISR Observations

    NASA Technical Reports Server (NTRS)

    Guo, Yanjuan; Tian, Baijun; Kahn, Ralph A.; Kalashnikova, Olga; Wong, Sun; Waliser, Duane E.

    2012-01-01

    In this study, MODIS fine mode fraction and MISR non-spherical fraction are 2used to derive dust and smoke AOT components (tau(sub dust) and tau(sub smoke)) over the tropical Atlantic, and their variabilities related to the Madden-Julian Oscillation (MJO) are then investigated. Both MODIS and MISR show a very similar dust and smoke winter climatology. tau(sub dust) is found to be the dominant aerosol component over the tropical Atlantic while tau(sub smoke) is significantly smaller than tau(sub dust). The daily MODIS and MISR tau(sub dust) are overall highly correlated, with the correlation coefficients typically about 0.7 over the North Atlantic. The consistency between the MODIS and MISR dust and smoke aerosol climatology and daily variations give us confidence to use these two data sets to investigate their relative contributions to the total AOT variation associated with the MJO. However, unlike the MISR dust discrimination, which is based on particle shape retrievals, the smoke discrimination is less certain, based on assumed partitioning of maritime aerosol for both MISR and MODIS. The temporal evolution and spatial patterns of the tau(sub dust) anomalies associated with the MJO are consistent between MODIS and MISR. The tau(sub dust) anomalies are very similar to those of tau anomalies, and are of comparable magnitude. In contrast, the MJO-related tau(sub smoke) anomalies are rather small, and the tau(sub mar) anomalies are negligible. The consistency between the MODIS and MISR results suggests that dust aerosol is the dominant component on the intra-seasonal time scale over the tropical Atlantic Ocean.

  14. Impact of Interactive Aerosol on the African Easterly Jet in the NASA GEOS-5 Global Forecasting System

    NASA Technical Reports Server (NTRS)

    Reale, O.; Lau, K. M.; da Silva, A.

    2010-01-01

    The real-time treatment of interactive realistically varying aerosol in a global operational forecasting system, as opposed to prescribed (fixed or climatologically varying) aerosols, is a very difficult challenge that only recently begins to be addressed. Experiment results from a recent version of the NASA GEOS-5 forecasting system, inclusive of interactive aerosol treatment, are presented in this work. Four sets of 30 5-day forecasts are initialized from a high quality set of analyses previously produced and documented to cover the period from 15 August to 16 September 2006, which corresponds to the NASA African Monsoon Multidisciplinary Analysis (NAMMA) observing campaign. The four forecast sets are at two different horizontal resolutions and with and without interactive aerosol treatment. The net impact of aerosol, at times in which there is a strong dust outbreak, is a temperature increase at the dust level and decrease in the near-surface levels, in complete agreement with previous observational and modeling studies. Moreover, forecasts in which interactive aerosols are included depict an African Easterly (AEJ) at slightly higher elevation, and slightly displace northward, with respect to the forecasts in which aerosols are not include. The shift in the AEJ position goes in the direction of observations and agrees with previous results.

  15. Response to Toward Unified Satellite Climatology of Aerosol Properties. 3; MODIS versus MISR versus AERONET

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.; Garay, Michael J.; Nelson, David L.; Levy, Robert C.; Bull, Michael A.; Diner, David J.; Martonchik, John V.; Hansen, Earl G.; Remer, Lorraine A.; Tanre, Didler

    2010-01-01

    A recent paper by Mishchenko et al. compares near-coincident MISR, MODIS, and AERONET aerosol optical depth (AOD), and gives a much less favorable impression of the utility of the satellite products than that presented by the instrument teams and other groups. We trace the reasons for the differing pictures to whether known and previously documented limitations of the products are taken into account in the assessments. Specifically, the analysis approaches differ primarily in (1) the treatment of outliers, (2) the application of absolute vs. relative criteria for testing agreement, and (3) the ways in which seasonally varying spatial distributions of coincident retrievals are taken into account. Mishchenko et al. also do not distinguish between observational sampling differences and retrieval algorithm error. We assess the implications of the different analysis approaches, and cite examples demonstrating how the MISR and MODIS aerosol products have been applied successfully to a range of scientific investigations.

  16. NASA/GEWEX shortwave surface radiation budget: Integrated data product with reprocessed radiance, cloud, and meteorology inputs, and new surface albedo treatment

    NASA Astrophysics Data System (ADS)

    Cox, Stephen J.; Stackhouse, Paul W.; Gupta, Shashi K.; Mikovitz, J. Colleen; Zhang, Taiping

    2017-02-01

    The NASA/GEWEX Surface Radiation Budget (SRB) project produces shortwave and longwave surface and top of atmosphere radiative fluxes for the 1983-near present time period. Spatial resolution is 1 degree. The current Release 3.0 (available at gewex-srb.larc.nasa.gov) uses the International Satellite Cloud Climatology Project (ISCCP) DX product for pixel level radiance and cloud information. This product is subsampled to 30 km. ISCCP is currently recalibrating and recomputing their entire data series, to be released as the H product, at 10km resolution. The ninefold increase in pixel number will allow SRB a higher resolution gridded product (e.g. 0.5 degree), as well as the production of pixel-level fluxes. Other key input improvements include a detailed aerosol history using the Max Planck Institute Aerosol Climatology (MAC), and temperature and moisture profiles from nnHIRS.

  17. Sensitivity of Boreal-Summer Circulation and Precipitation to Atmospheric Aerosols in Selected Regions: Part I Africa and India

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Sud, Yogesh C.; Wilcox, Eric; Lau, William K.

    2009-10-23

    Version-4 of the Goddard Earth Observing System (GEOS-4) General Circulation Model (GCM) was employed to assess the influence of potential changes in aerosols on the regional circulation, ambient temperatures, and precipitation in four selected regions: India and Africa (current paper), as well as North and South America (companion paper). Ensemble-simulations were carried out with the GCM to assess the aerosol direct and indirect effects, hereafter ADE and AIE. Each simulation was started from the NCEP-analyzed initial conditions for May 1 and was integrated through May-June-July-August of each year: 1982-1987 to provide an ensemble set of six simulations. In the firstmore » set, called the baseline experiment (#1), climatological aerosols were prescribed. The next two experiments (#2 and #3) had two sets of simulations each: one with 2X and another with 1/2X the climatological aerosols over each of the four selected regions. In experiment#2, the anomaly regions were advectively restricted (AR), i.e., the large-scale prognostic fields outside the aerosol anomaly regions were prescribed while in experiment#3, the anomaly regions were advectively Interactive (AI) as is the case in a normal GCM integrations, but with the same aerosols anomalies as in experiment #2. Intercomparisons of circulation, diabatic heating, and precipitation difference fields showed large disparities among the AR and AI simulations, which raised serious questions about the AR assumption, commonly invoked in regional climate simulation studies. Consequently AI simulation mode was chosen for the subsequent studies. Two more experiments (#4 and #5) were performed in the AI mode in which ADE and AIE were activated one at a time. The results showed that ADE and AIE work in concert to make the joint influences larger than sum of each acting alone. Moreover, the ADE and AIE influences were vastly different for the Indian and Africa regions, which suggest an imperative need to include them

  18. On the Analysis of the Climatology of Cloudiness of the Arabian Peninsula

    NASA Astrophysics Data System (ADS)

    Yousef, L. A.; Temimi, M.

    2015-12-01

    This study aims to determine the climatology of cloudiness over the Arabian Peninsula. The determined climatology will assist solar energy resource assessment in the region. The seasonality of cloudiness and its spatial variability will also help guide several cloud seeding operational experiments in the region. Cloud properties from the International Satellite Cloud Climatology Project (ISCCP) database covering the time period from 1983 through 2009 are analyzed. Time series of low, medium, high, and total cloud amounts are investigated, in addition to cloud optical depth and total column water vapor. Initial results show significant decreasing trends in the total and middle cloud amounts, both annually and seasonally, at a 95% confidence interval. The relationship between cloud amounts and climate oscillations known to affect the region is explored. Climate indices exhibiting significant correlations with the total cloud amounts include the Pacific Decadal Oscillation (PDO) index. The study also includes a focus on the United Arab Emirates (UAE), comparing the inferred cloudiness data to in situ rainfall measurements taken from rain gauges across the UAE. To assess the impact of cloudiness on solar power resources in the country, time series of cloud amounts and Direct Normal Irradiance (DNI), obtained from the UAE Solar Atlas, are compared.

  19. Constructing an AIRS Climatology for Data Visualization and Analysis to Serve the Climate Science and Application Communities

    NASA Technical Reports Server (NTRS)

    Ding, Feng; Keim, Elaine; Hearty, Thomas J.; Wei, Jennifer; Savtchenko, Andrey; Theobald, Michael; Vollmer, Bruce

    2016-01-01

    The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) is the home of processing, archiving, and distribution services for NASA sounders: the present Aqua AIRS mission and the succeeding SNPP CrIS mission. The AIRS mission is entering its 15th year of global observations of the atmospheric state, including temperature and humidity profiles, outgoing longwave radiation, cloud properties, and trace gases. The GES DISC, in collaboration with the AIRS Project, released product from the version 6 algorithm in early 2013. Giovanni, a Web-based application developed by the GES DISC, provides a simple and intuitive way to visualize, analyze, and access vast amounts of Earth science remote sensing data without having to download the data. Most important variables from version 6 AIRS product are available in Giovanni. We are developing a climatology product using 14-year AIRS retrievals. The study can be a good start for the long term climatology from NASA sounders: the AIRS and the succeeding CrIS. This presentation will show the impacts to the climatology product from different aggregation methods. The climatology can serve climate science and application communities in data visualization and analysis, which will be demonstrated using a variety of functions in version 4 Giovanni. The highlights of these functions include user-defined monthly and seasonal climatology, inter annual seasonal time series, anomaly analysis.

  20. Constructing an AIRS Climatology for Data Visualization and Analysis to Serve the Climate Science and Application Communities

    NASA Astrophysics Data System (ADS)

    Ding, F.; Keim, E.; Hearty, T. J., III; Wei, J. C.; Savtchenko, A.; Theobald, M.; Vollmer, B.

    2016-12-01

    The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) is the home of processing, archiving, and distribution services for NASA sounders: the present Aqua AIRS mission and the succeeding SNPP CrIS mission. The AIRS mission is entering its 15th year of global observations of the atmospheric state, including temperature and humidity profiles, outgoing longwave radiation, cloud properties, and trace gases. The GES DISC, in collaboration with the AIRS Project, released product from the version 6 algorithm in early 2013. Giovanni, a Web-based application developed by the GES DISC, provides a simple and intuitive way to visualize, analyze, and access vast amounts of Earth science remote sensing data without having to download the data. Most important variables from version 6 AIRS product are available in Giovanni. We are developing a climatology product using 14-year AIRS retrievals. The study can be a good start for the long term climatology from NASA sounders: the AIRS and the succeeding CrIS. This presentation will show the impacts to the climatology product from different aggregation methods. The climatology can serve climate science and application communities in data visualization and analysis, which will be demonstrated using a variety of functions in version 4 Giovanni. The highlights of these functions include user-defined monthly and seasonal climatology, inter annual seasonal time series, anomaly analysis.

  1. The International Satellite Cloud Climatology Project H-Series climate data record product

    NASA Astrophysics Data System (ADS)

    Young, Alisa H.; Knapp, Kenneth R.; Inamdar, Anand; Hankins, William; Rossow, William B.

    2018-03-01

    This paper describes the new global long-term International Satellite Cloud Climatology Project (ISCCP) H-series climate data record (CDR). The H-series data contain a suite of level 2 and 3 products for monitoring the distribution and variation of cloud and surface properties to better understand the effects of clouds on climate, the radiation budget, and the global hydrologic cycle. This product is currently available for public use and is derived from both geostationary and polar-orbiting satellite imaging radiometers with common visible and infrared (IR) channels. The H-series data currently span July 1983 to December 2009 with plans for continued production to extend the record to the present with regular updates. The H-series data are the longest combined geostationary and polar orbiter satellite-based CDR of cloud properties. Access to the data is provided in network common data form (netCDF) and archived by NOAA's National Centers for Environmental Information (NCEI) under the satellite Climate Data Record Program (https://doi.org/10.7289/V5QZ281S). The basic characteristics, history, and evolution of the dataset are presented herein with particular emphasis on and discussion of product changes between the H-series and the widely used predecessor D-series product which also spans from July 1983 through December 2009. Key refinements included in the ISCCP H-series CDR are based on improved quality control measures, modified ancillary inputs, higher spatial resolution input and output products, calibration refinements, and updated documentation and metadata to bring the H-series product into compliance with existing standards for climate data records.

  2. Climatological determinants of woody cover in Africa.

    PubMed

    Good, Stephen P; Caylor, Kelly K

    2011-03-22

    Determining the factors that influence the distribution of woody vegetation cover and resolving the sensitivity of woody vegetation cover to shifts in environmental forcing are critical steps necessary to predict continental-scale responses of dryland ecosystems to climate change. We use a 6-year satellite data record of fractional woody vegetation cover and an 11-year daily precipitation record to investigate the climatological controls on woody vegetation cover across the African continent. We find that-as opposed to a relationship with only mean annual rainfall-the upper limit of fractional woody vegetation cover is strongly influenced by both the quantity and intensity of rainfall events. Using a set of statistics derived from the seasonal distribution of rainfall, we show that areas with similar seasonal rainfall totals have higher fractional woody cover if the local rainfall climatology consists of frequent, less intense precipitation events. Based on these observations, we develop a generalized response surface between rainfall climatology and maximum woody vegetation cover across the African continent. The normalized local gradient of this response surface is used as an estimator of ecosystem vegetation sensitivity to climatological variation. A comparison between predicted climate sensitivity patterns and observed shifts in both rainfall and vegetation during 2009 reveals both the importance of rainfall climatology in governing how ecosystems respond to interannual fluctuations in climate and the utility of our framework as a means to forecast continental-scale patterns of vegetation shifts in response to future climate change.

  3. Microphysical Cloud Regimes used as a tool to study Aerosol-Cloud-Precipitation-Radiation interactions

    NASA Astrophysics Data System (ADS)

    Cho, N.; Oreopoulos, L.; Lee, D.

    2017-12-01

    The presentation will examine whether the diagnostic relationships between aerosol and cloud-affected quantities (precipitation, radiation) obtained from sparse temporal resolution measurements from polar orbiting satellites can potentially demonstrate actual aerosol effects on clouds with appropriate analysis. The analysis relies exclusively on Level-3 (gridded) data and comprises systematic cloud classification in terms of "microphysical cloud regimes" (µCRs), aerosol optical depth (AOD) variations relative to a region's local seasonal climatology, and exploitation of the 3-hour difference between Terra (morning) and Aqua (afternoon) overpasses. Specifically, our presentation will assess whether Aerosol-Cloud-Precipitation-Radiation interactions (ACPRI) can be diagnosed by investigating: (a) The variations with AOD of afternoon cloud-affected quantities composited by afternoon or morning µCRs; (b) µCR transition diagrams composited by morning AOD quartiles; (c) whether clouds represented by ensemble cloud effective radius - cloud optical thickness joint histograms look distinct under low and high AOD conditions when preceded or followed by specific µCRs. We will explain how our approach addresses long-standing themes of the ACPRI problem such as the optimal ways to decompose the problem by cloud class, the prevalence and detectability of 1st/2nd aerosol indirect effects and invigoration, and the effectiveness of aerosol changes in inducing cloud modification at different segments of the AOD distribution.

  4. Ozone Climatological Profiles for Version 8 TOMS and SBUV Retrievals

    NASA Technical Reports Server (NTRS)

    McPeters, R. D.; Logan, J. A.; Labow, G. J.

    2003-01-01

    A new altitude dependent ozone climatology has been produced for use with the latest Total Ozone Mapping Spectrometer (TOMS) and Solar Backscatter Ultraviolet (SBUV) retrieval algorithms. The climatology consists of monthly average profiles for ten degree latitude zones covering from 0 to 60 km. The climatology was formed by combining data from SAGE II (1988 to 2000) and MLS (1991-1999) with data from balloon sondes (1988-2002). Ozone below about 20 km is based on balloons sondes, while ozone above 30 km is based on satellite measurements. The profiles join smoothly between 20 and 30 km. The ozone climatology in the southern hemisphere and tropics has been greatly enhanced in recent years by the addition of balloon sonde stations under the SHADOZ (Southern Hemisphere Additional Ozonesondes) program. A major source of error in the TOMS and SBUV retrieval of total column ozone comes from their reduced sensitivity to ozone in the lower troposphere. An accurate climatology for the retrieval a priori is important for reducing this error on the average. The new climatology follows the seasonal behavior of tropospheric ozone and reflects its hemispheric asymmetry. Comparisons of TOMS version 8 ozone with ground stations show an improvement due in part to the new climatology.

  5. An Updated TRMM Composite Climatology of Tropical Rainfall and Its Validation

    NASA Technical Reports Server (NTRS)

    Wang, Jian-Jian; Adler, Robert F.; Huffman, George; Bolvin, David

    2013-01-01

    An updated 15-yr Tropical Rainfall Measuring Mission (TRMM) composite climatology (TCC) is presented and evaluated. This climatology is based on a combination of individual rainfall estimates made with data from the primaryTRMMinstruments: theTRMM Microwave Imager (TMI) and the precipitation radar (PR). This combination climatology of passive microwave retrievals, radar-based retrievals, and an algorithm using both instruments simultaneously provides a consensus TRMM-based estimate of mean precipitation. The dispersion of the three estimates, as indicated by the standard deviation sigma among the estimates, is presented as a measure of confidence in the final estimate and as an estimate of the uncertainty thereof. The procedures utilized by the compositing technique, including adjustments and quality-control measures, are described. The results give a mean value of the TCC of 4.3mm day(exp -1) for the deep tropical ocean beltbetween 10 deg N and 10 deg S, with lower values outside that band. In general, the TCC values confirm ocean estimates from the Global Precipitation Climatology Project (GPCP) analysis, which is based on passive microwave results adjusted for sampling by infrared-based estimates. The pattern of uncertainty estimates shown by sigma is seen to be useful to indicate variations in confidence. Examples include differences between the eastern and western portions of the Pacific Ocean and high values in coastal and mountainous areas. Comparison of the TCC values (and the input products) to gauge analyses over land indicates the value of the radar-based estimates (small biases) and the limitations of the passive microwave algorithm (relatively large biases). Comparison with surface gauge information from western Pacific Ocean atolls shows a negative bias (16%) for all the TRMM products, although the representativeness of the atoll gauges of open-ocean rainfall is still in question.

  6. Recent Progress on Deep Blue Aerosol Algorithm as Applied TO MODIS, SEA WIFS, and VIIRS, and Their Intercomparisons with Ground Based and Other Satellite Measurements

    NASA Technical Reports Server (NTRS)

    Hsu, N. Christina; Bettenhausen, Corey; Sawyer, Andrew; Tsay, Si-Chee

    2012-01-01

    The impact of natural and anthropogenic sources of aerosols has gained increasing attention from scientific communities in recent years. Indeed, tropospheric aerosols not only perturb radiative energy balance by interacting with solar and terrestrial radiation, but also by changing cloud properties and lifetime. Furthermore, these anthropogenic and natural air particles, once generated over the source regions, can be transported out of the boundary layer into the free troposphere and can travel thousands of kilometers across oceans and continents resulting in important biogeochemical impacts on the ecosystem. With the launch of SeaWiFS in 1997, Terra/MODIS in 1999, and Aqua/MODIS in 2002, high quality comprehensive aerosol climatology is becoming feasible for the first time. As a result of these unprecedented data records, studies of the radiative and biogeochemical effects due to tropospheric aerosols are now possible. In this talk, we will demonstrate how this newly available SeaWiFS/MODIS aerosol climatology can provide an important piece of puzzles in reducing the uncertainty of estimated climatic forcing due to aerosols. We will start with the global distribution of aerosol loading and their variabilities over both land and ocean on short- and long-term temporal scales observed over the last decade. The recent progress made in Deep Blue aerosol algorithm on improving accuracy of these Sea WiFS / MODIS aerosol products in particular over land will be discussed. The impacts on quantifying physical and optical processes of aerosols over source regions of adding the Deep Blue products of aerosol properties over bright-reflecting surfaces into Sea WiFS / MODIS as well as VIIRS data suite will also be addressed. We will also show the intercomparison results of SeaWiFS/MODIS retrieved aerosol optical thickness with data from ground based AERONET sunphotometers over land and ocean as well as with other satellite measurements. The trends observed in global aerosol

  7. A Ten-Year Global Record of Absorbing Aerosols Above Clouds from OMI's Near-UV Observations

    NASA Technical Reports Server (NTRS)

    Jethva, Hiren; Torres, Omar; Ahn, Changwoo

    2016-01-01

    Aerosol-cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of an adequate knowledge of the complex microphysical and radiative processes associated with the aerosol-cloud system. The situations when aerosols and clouds are found in the same atmospheric column, for instance, when light-absorbing aerosols such as biomass burning generated carbonaceous particles or wind-blown dust overlay low-level cloud decks, are commonly found over several regional of the world. Contrary to the cloud-free scenario over dark surface, for which aerosols are known to produce a net cooling effect (negative radiative forcing) on climate, the overlapping situation of absorbing aerosols over cloud can potentially exert a significant level of atmospheric absorption and produces a positive radiative forcing at top-of-atmosphere. The magnitude of direct radiative effects of aerosols above cloud depends directly on the aerosol loading, microphysical-optical properties of the aerosol layer and the underlying cloud deck, and geometric cloud fraction. We help in addressing this problem by introducing a novel product of optical depth of absorbing aerosols above clouds retrieved from near-UV observations made by the Ozone Monitoring Instrument (OMI) on board NASA's Aura platform. The presence of absorbing aerosols above cloud reduces the upwelling radiation reflected by cloud and produces a strong 'color ratio' effect in the near-UV region, which can be unambiguously detected in the OMI measurements. Physically based on this effect, the OMACA algorithm retrieves the optical depths of aerosols and clouds simultaneously under a prescribed state of atmosphere. The algorithm architecture and results from a ten-year global record including global climatology of frequency of occurrence and above-cloud aerosol optical depth, and a discussion on related future field campaigns are presented.

  8. Observations and projections of visibility and aerosol optical thickness (1956-2100) in the Netherlands: impacts of time-varying aerosol composition and hygroscopicity

    NASA Astrophysics Data System (ADS)

    Boers, R.; van Weele, M.; van Meijgaard, E.; Savenije, M.; Siebesma, A. P.; Bosveld, F.; Stammes, P.

    2015-01-01

    Time series of visibility and aerosol optical thickness for the Netherlands have been constructed for 1956-2100 based on observations and aerosol mass scenarios. Aerosol optical thickness from 1956 to 2013 has been reconstructed by converting time series of visibility to visible extinction which in turn are converted to aerosol optical thickness using an appropriate scaling depth. The reconstruction compares closely with remote sensing observations of aerosol optical thickness between 1960 and 2013. It appears that aerosol optical thickness was relatively constant over the Netherlands in the years 1955-1985. After 1985, visibility has improved, while at the same time aerosol optical thickness has decreased. Based on aerosol emission scenarios for the Netherlands three aerosol types have been identified: (1) a constant background consisting of sea salt and mineral dust, (2) a hydrophilic anthropogenic inorganic mixture, and (3) a partly hydrophobic mixture of black carbon (BC) and organic aerosols (OAs). A reduction in overall aerosol concentration turns out to be the most influential factor in the reduction in aerosol optical thickness. But during 1956-1985, an upward trend in hydrophilic aerosols and associated upward trend in optical extinction has partly compensated the overall reduction in optical extinction due to the reduction in less hydrophilic BC and OAs. A constant optical thickness ensues. This feature highlights the influence of aerosol hygroscopicity on time-varying signatures of atmospheric optical properties. Within the hydrophilic inorganic aerosol mixture there is a gradual shift from sulfur-based (1956-1985) to a nitrogen-based water aerosol chemistry (1990 onwards) but always modulated by the continual input of sodium from sea salt. From 2013 to 2100, visibility is expected to continue its increase, while at the same time optical thickness is foreseen to continue to decrease. The contribution of the hydrophilic mixture to the aerosol optical

  9. Investigating the Impact of Aerosol Deposition on Snow Melt over the Greenland Ice Sheet Using a New Kernel

    NASA Astrophysics Data System (ADS)

    Li, Y.; Flanner, M.

    2017-12-01

    Accelerating surface melt on the Greenland Ice Sheet (GrIS) has led to a doubling of Greenland's contribution to global sea level rise during recent decades. The darkening effect due to black carbon (BC), dust, and other light absorbing impurities (LAI) enhances snow melt by boosting its absorption of solar energy. It is therefore important for coupled aerosol-climate and ice sheet models to include snow darkening effects from LAI, and yet most do not. In this study, we develop an aerosol deposition—snow melt kernel based on the Community Earth System Model (CESM) to investigate changes in melt flux due to variations in the amount and timing of aerosol deposition on the GrIS. The Community Land Model (CLM) component of CESM is driven with a large range of aerosol deposition fluxes to determine non-linear relationships between melt perturbation and deposition amount occurring in different months and location (thereby capturing variations in base state associated with elevation and latitude). The kernel product will include climatological-mean effects and standard deviations associated with interannual variability. Finally, the kernel will allow aerosol deposition fluxes from any global or regional aerosol model to be translated into surface melt perturbations of the GrIS, thus extending the utility of state-of-the-art aerosol models.

  10. Preliminary aerosol generator design studies

    NASA Technical Reports Server (NTRS)

    Stampfer, J. F., Jr.

    1976-01-01

    The design and construction of a prototype vaporization generator for highly dispersed sodium chloride aerosols is described. The aerosol generating system is to be used in the Science Simulator of the Cloud Physics Laboratory Project and as part of the Cloud Physics Laboratory payload to be flown on the shuttle/spacelab.

  11. Importance of Anthropogenic Aerosols for Climate Prediction: a Study on East Asian Sulfate Aerosols

    NASA Astrophysics Data System (ADS)

    Bartlett, R. E.; Bollasina, M. A.

    2017-12-01

    Climate prediction is vital to ensure that we are able to adapt to our changing climate. Understandably, the main focus for such prediction is greenhouse gas forcing, as this will be the main anthropogenic driver of long-term global climate change; however, other forcings could still be important. Atmospheric aerosols represent one such forcing, especially in regions with high present-day aerosol loading such as Asia; yet, uncertainty in their future emissions are under-sampled by commonly used climate forcing projections, such as the Representative Concentration Pathways (RCPs). Globally, anthropogenic aerosols exert a net cooling, but their effects show large variation at regional scales. Studies have shown that aerosols impact locally upon temperature, precipitation and hydroclimate, and also upon larger scale atmospheric circulation (for example, the Asian monsoon) with implications for climate remote from aerosol sources. We investigate how future climate could evolve differently given the same greenhouse gas forcing pathway but differing aerosol emissions. Specifically, we use climate modelling experiments (using HadGEM2-ES) of two scenarios based upon RCP2.6 greenhouse gas forcing but with large differences in sulfur dioxide emissions over East Asia. Results show that increased sulfate aerosols (associated with increased sulfur dioxide) lead to large regional cooling through aerosol-radiation and aerosol-cloud interactions. Focussing on dynamical mechanisms, we explore the consequences of this cooling for the Asian summer and winter monsoons. In addition to local temperature and precipitation changes, we find significant changes to large scale atmospheric circulation. Wave-like responses to upper-level atmospheric changes propagate across the northern hemisphere with far-reaching effects on surface climate, for example, cooling over Europe. Within the tropics, we find alterations to zonal circulation (notably, shifts in the Pacific Walker cell) and monsoon

  12. The response of European and Asian climate to global and regional aerosol emissions

    NASA Astrophysics Data System (ADS)

    Wilcox, Laura; Dunstone, Nick; Highwood, Eleanor; Bollasina, Massimo; Dong, Buwen; Sutton, Rowan

    2017-04-01

    Asia has the world's highest anthropogenic aerosol loading and has experienced a dramatic increase in emissions since the 1950s, which has continued in the 21st century, in stark contrast with European (and North American) emissions which started to decrease in the 1970s. We use a set of transient coupled model experiments (HadGEM2-GC2) to explore the regional climate effects of anthropogenic aerosol changes since the 1980s, with a focus on the European and Asian responses. Comparing simulations with globally varying aerosol emissions to an equivalent set with Asian emissions fixed at their 1971-1980 mean over Asia, we identify the contribution of Asian emissions to the total impact. Identifying thermodynamic and dynamic responses to global and regional aerosol changes, we diagnose atmospheric teleconnections and their interactions with local processes, and the mechanisms by which aerosol affects both European and Asian climate. It is found that Asian aerosols led to substantial changes in Asian climate, weakening the summer monsoon, which is a key driver of the observed precipitation changes there in recent decades. Asian emissions are also able to induce planetary-scale teleconnection patterns in both winter and summer. The impact of the regional diabatic heating anomaly propagates remotely by exciting northern hemisphere wave-trains which, enhanced by regional feedbacks, cause changes in near-surface climate over Europe. To examine the robustness of the mechanisms we identify in HadGEM2, we analyse similar sets of experiments from NorESM1-M and GFDL-CM3: models with very different climatologies and representations of aerosol processes.

  13. Spherical harmonic analysis of a model-generated climatology

    NASA Technical Reports Server (NTRS)

    Christidis, Z. D.; Spar, J.

    1981-01-01

    Monthly mean fields of 850 mb temperature (T850), 500 mb geopotential height (G500) and sea level pressure (SLP) were generated in the course of a five-year climate simulation run with a global general circulation model. Both the model-generated climatology and an observed climatology were subjected to spherical harmonic analysis, with separate analyses of the globe and the Northern Hemisphere. Comparison of the dominant harmonics of the two climatologies indicates that more than 95% of the area-weighted spatial variance of G500 and more than 90% of that of T850 are explained by fewer than three components, and that the model adequately simulates these large-scale characteristics. On the other hand, as many as 25 harmonics are needed to explain 95% of the observed variance of SLP, and the model simulation of this field is much less satisfactory. The model climatology is also evaluated in terms of the annual cycles of the dominant harmonics.

  14. Airborne Cavity Ring-Down Measurement of Aerosol Extinction and Scattering During the Aerosol IOP

    NASA Technical Reports Server (NTRS)

    Strawa, A. W.; Ricci, K.; Provencal, R.; Schmid, B.; Covert, D.; Elleman, R.; Arnott, P.

    2003-01-01

    Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300 Mm-1 with an estimated precision of 0.1 Min-1 for 1550 nm light and 0.2 Mm-1 for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects.= We present comparisons between the Cadenza measurements and those friom a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS 14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

  15. Detect signals of interdecadal climate variations from an enhanced suite of reconstructed precipitation products since 1850 using the historical station data from Global Historical Climatology Network and the dynamical patterns derived from Global Precipitation Climatology Project

    NASA Astrophysics Data System (ADS)

    Shen, S. S.

    2015-12-01

    This presentation describes the detection of interdecadal climate signals in a newly reconstructed precipitation data from 1850-present. Examples are on precipitation signatures of East Asian Monsoon (EAM), Pacific Decadal Oscillation (PDO) and Atlantic Multidecadal Oscillations (AMO). The new reconstruction dataset is an enhanced edition of a suite of global precipitation products reconstructed by Spectral Optimal Gridding of Precipitation Version 1.0 (SOGP 1.0). The maximum temporal coverage is 1850-present and the spatial coverage is quasi-global (75S, 75N). This enhanced version has three different temporal resolutions (5-day, monthly, and annual) and two different spatial resolutions (2.5 deg and 5.0 deg). It also has a friendly Graphical User Interface (GUI). SOGP uses a multivariate regression method using an empirical orthogonal function (EOF) expansion. The Global Precipitation Climatology Project (GPCP) precipitation data from 1981-20010 are used to calculate the EOFs. The Global Historical Climatology Network (GHCN) gridded data are used to calculate the regression coefficients for reconstructions. The sampling errors of the reconstruction are analyzed according to the number of EOF modes used in the reconstruction. Our reconstructed 1900-2011 time series of the global average annual precipitation shows a 0.024 (mm/day)/100a trend, which is very close to the trend derived from the mean of 25 models of the CMIP5 (Coupled Model Intercomparison Project Phase 5). Our reconstruction has been validated by GPCP data after 1979. Our reconstruction successfully displays the 1877 El Nino (see the attached figure), which is considered a validation before 1900. Our precipitation products are publically available online, including digital data, precipitation animations, computer codes, readme files, and the user manual. This work is a joint effort of San Diego State University (Sam Shen, Gregori Clarke, Christian Junjinger, Nancy Tafolla, Barbara Sperberg, and

  16. Toward Unified Satellite Climatology of Aerosol Properties. 3. MODIS Versus MISR Versus AERONET

    NASA Technical Reports Server (NTRS)

    Mishchenko, Michael I.; Liu, Li; Geogdzhayev, Igor V.; Travis, Larry D.; Cairns, Brian; Lacis, Andrew A.

    2010-01-01

    We use the full duration of collocated pixel-level MODIS-Terra and MISR aerosol optical thickness (AOT) retrievals and level 2 cloud-screened quality-assured AERONET measurements to evaluate the likely individual MODIS and MISR retrieval accuracies globally over oceans and land. We show that the use of quality-assured MODIS AOTs as opposed to the use of all MODIS AOTs has little effect on the resulting accuracy. The MODIS and MISR relative standard deviations (RSTDs) with respect to AERONET are remarkably stable over the entire measurement record and reveal nearly identical overall AOT performances of MODIS and MISR over the entire suite of AERONET sites. This result is used to evaluate the likely pixel-level MODIS and MISR performances on the global basis with respect to the (unknown) actual AOTs. For this purpose, we use only fully compatible MISR and MODIS aerosol pixels. We conclude that the likely RSTDs for this subset of MODIS and MISR AOTs are 73% over land and 30% over oceans. The average RSTDs for the combined [AOT(MODIS)+AOT(MISR)]/2 pixel-level product are close to 66% and 27%, respectively, which allows us to recommend this simple blend as a better alternative to the original MODIS and MISR data. These accuracy estimates still do not represent the totality of MISR and quality-assured MODIS pixel-level AOTs since an unaccounted for and potentially significant source of errors is imperfect cloud screening. Furthermore, many collocated pixels for which one of the datasets reports a retrieval, whereas the other one does not may also be problematic.

  17. Long-term trend analysis and climatology of tropical cirrus clouds using 16 years of lidar data set over Southern India

    NASA Astrophysics Data System (ADS)

    Pandit, A. K.; Gadhavi, H. S.; Venkat Ratnam, M.; Raghunath, K.; Rao, S. V. B.; Jayaraman, A.

    2015-12-01

    Sixteen-year (1998-2013) climatology of cirrus clouds and their macrophysical (base height, top height and geometrical thickness) and optical properties (cloud optical thickness) observed using a ground-based lidar over Gadanki (13.5° N, 79.2° E), India, is presented. The climatology obtained from the ground-based lidar is compared with the climatology obtained from 7 and a half years (June 2006-December 2013) of Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) observations. A very good agreement is found between the two climatologies in spite of their opposite viewing geometries and the differences in sampling frequencies. Nearly 50-55 % of cirrus clouds were found to possess geometrical thickness less than 2 km. Ground-based lidar is found to detect a higher number of sub-visible clouds than CALIOP which has implications for global warming studies as sub-visible cirrus clouds have significant positive radiative forcing. Cirrus clouds with mid-cloud temperatures between -50 to -70 °C have a mean geometrical thickness greater than 2 km in contrast to the earlier reported value of 1.7 km. Trend analyses reveal a statistically significant increase in the altitude of sub-visible cirrus clouds which is consistent with the recent climate model simulations. The mid-cloud altitude of sub-visible cirrus clouds is found to be increasing at the rate of 41 ± 21 m year-1. Statistically significant decrease in optical thickness of sub-visible and thick cirrus clouds is observed. Also, the fraction of sub-visible cirrus cloud is found to have increased by 9 % in the last 16 years (1998 to 2013). This increase is mainly compensated by a 7 % decrease in thin cirrus cloud fraction. This has implications for the temperature and water vapour budget in the tropical tropopause layer.

  18. Ambient Aerosol in Southeast Asia: High Resolution Aerosol Mass Spectrometer Measurements Over Oil Palm (Elaeis guineensis)

    NASA Astrophysics Data System (ADS)

    Phillips, G.; Dimarco, C.; Misztal, P.; Nemitz, E.; Farmer, D.; Kimmel, J.; Jimenez, J.

    2008-12-01

    The emission of organic compounds in the troposphere is important factor in the formation of secondary organic aerosol (SOA). A very large proportion of organic material emitted globally is estimated to arise from biogenic sources, with almost half coming from tropical and sub-tropical forests. Preliminary analyses of leave cuvette emission studies suggest that oil palm (Elaeis guineensis) is a significantly larger source of isoprene than tropical forest. Much larger sources of isoprene over oil palm allied with a larger anthropogenic component of local emissions contrast greatly with the remote tropical forest environment and therefore the character of SOA formed may differ significantly. These issues, allied with the high price of palm oil on international markets leading to increased use of land for oil palm production, could give rise to rapidly changing chemical and aerosol regimes in the tropics. It is therefore important to understand the current emissions and composition of organic aerosol over all important land-uses in the tropical environment. This in turn will lead to a greater understanding of the present, and to an improvement in predictive capacity for the future system. To help address these issues, a high resolution time of flight aerosol mass spectrometer (HR-ToF-AMS) was deployed in the Sabahmas (PPB OIL) oil palm plantation near Lahad Datu, in Eastern Sabah, as part of the field component of the Aerosol Coupling in the Earth System (ACES) project, part of the UK NERC APPRAISE program. This project was allied closely with measurements made of similar chemical species and aerosol components at a forest site in the Danum Valley as part of the UK Oxidant and Particle Photochemical Processes above a Southeast Asian tropical rainforest (OP3) project. Measurements of submicron non- refractory aerosol composition are presented along with some preliminary analysis of chemically resolved aerosol fluxes made with a new eddy covariance system, based on the

  19. A Satellite-based Assessment of Trans-Pacific Transport of Pollution Aerosol

    NASA Technical Reports Server (NTRS)

    Yu, Hongbin; Remer, Lorraine; Chin, Mian; Bian, Huisheng; Kleidman, Richard; Diehl. Thomas

    2007-01-01

    It has been well documented that pollution aerosol and dust from East Asia can transport across the North Pacific basin, reaching North America and beyond. Such intercontinental transport extends the impact of aerosols for climate change, air quality, atmospheric chemistry, and ocean biology from local and regional scales to hemispheric and global scales. Long term, measurement-based studies are necessary to adequately assess the implications of these wider impacts. A satellite-based assessment can augment intensive field campaigns by expanding temporal and spatial scales and also serve as constraints for model simulations. Satellite imagers have been providing a wealth of evidence for the intercontinental transport of aerosols for more than two decades. Quantitative assessments, however, became feasible only recently as a result of the much improved measurement accuracy and enhanced new capabilities of satellite sensors. In this study, we generated a 4-year (2002 to 2005) climatology of optical depth for pollution aerosol (defined as a mixture of aerosols from urbanlindustrial pollution and biomass burning in this study) over the North Pacific from MODerate resolution Imaging Spectro-radiometer (MODIS) observations of fine- and coarse-mode aerosol optical depths. The pollution aerosol mass loading and fluxes were then calculated using measurements of the dependence of aerosol mass extinction efficiency on relative humidity and of aerosol vertical distributions from field campaigns and available satellite observations in the region. We estimated that about 18 Tg/year pollution aerosol is exported from East Asia to the northwestern Pacific Ocean, of which about 25% reaches the west coast of North America. The pollution fluxes are largest in spring and smallest in summer. For the period we have examined the strongest export and import of pollution particulates occurred in 2003, due largely to record intense Eurasia wildfires in spring and summer. The overall

  20. Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Grandey, Benjamin S.; Lee, Hsiang-He; Wang, Chien

    Open-burning fires play an important role in the earth's climate system. In addition to contributing a substantial fraction of global emissions of carbon dioxide, they are a major source of atmospheric aerosols containing organic carbon, black carbon, and sulfate. These “fire aerosols” can influence the climate via direct and indirect radiative effects. In this study, we investigate these radiative effects and the hydrological fast response using the Community Atmosphere Model version 5 (CAM5). Emissions of fire aerosols exert a global mean net radiative effect of −1.0 W m −2, dominated by the cloud shortwave response to organic carbon aerosol. The net radiative effectmore » is particularly strong over boreal regions. Conventionally, many climate modelling studies have used an interannually invariant monthly climatology of emissions of fire aerosols. However, by comparing simulations using interannually varying emissions vs. interannually invariant emissions, we find that ignoring the interannual variability of the emissions can lead to systematic overestimation of the strength of the net radiative effect of the fire aerosols. Globally, the overestimation is +23 % (−0.2 W m −2). Regionally, the overestimation can be substantially larger. For example, over Australia and New Zealand the overestimation is +58 % (−1.2 W m −2), while over Boreal Asia the overestimation is +43 % (−1.9 W m −2). The systematic overestimation of the net radiative effect of the fire aerosols is likely due to the non-linear influence of aerosols on clouds. However, ignoring interannual variability in the emissions does not appear to significantly impact the hydrological fast response. In order to improve understanding of the climate system, we need to take into account the interannual variability of aerosol emissions.« less

  1. Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires

    DOE PAGES

    Grandey, Benjamin S.; Lee, Hsiang-He; Wang, Chien

    2016-11-23

    Open-burning fires play an important role in the earth's climate system. In addition to contributing a substantial fraction of global emissions of carbon dioxide, they are a major source of atmospheric aerosols containing organic carbon, black carbon, and sulfate. These “fire aerosols” can influence the climate via direct and indirect radiative effects. In this study, we investigate these radiative effects and the hydrological fast response using the Community Atmosphere Model version 5 (CAM5). Emissions of fire aerosols exert a global mean net radiative effect of −1.0 W m −2, dominated by the cloud shortwave response to organic carbon aerosol. The net radiative effectmore » is particularly strong over boreal regions. Conventionally, many climate modelling studies have used an interannually invariant monthly climatology of emissions of fire aerosols. However, by comparing simulations using interannually varying emissions vs. interannually invariant emissions, we find that ignoring the interannual variability of the emissions can lead to systematic overestimation of the strength of the net radiative effect of the fire aerosols. Globally, the overestimation is +23 % (−0.2 W m −2). Regionally, the overestimation can be substantially larger. For example, over Australia and New Zealand the overestimation is +58 % (−1.2 W m −2), while over Boreal Asia the overestimation is +43 % (−1.9 W m −2). The systematic overestimation of the net radiative effect of the fire aerosols is likely due to the non-linear influence of aerosols on clouds. However, ignoring interannual variability in the emissions does not appear to significantly impact the hydrological fast response. In order to improve understanding of the climate system, we need to take into account the interannual variability of aerosol emissions.« less

  2. Situational Lightning Climatologies

    NASA Technical Reports Server (NTRS)

    Bauman, William; Crawford, Winifred

    2010-01-01

    Research has revealed distinct spatial and temporal distributions of lightning occurrence that are strongly influenced by large-scale atmospheric flow regimes. It was believed there were two flow systems, but it has been discovered that actually there are seven distinct flow regimes. The Applied Meteorology Unit (AMU) has recalculated the lightning climatologies for the Shuttle Landing Facility (SLF), and the eight airfields in the National Weather Service in Melbourne (NWS MLB) County Warning Area (CWA) using individual lightning strike data to improve the accuracy of the climatologies. The software determines the location of each CG lightning strike with 5-, 10-, 20-, and 30-nmi (.9.3-, 18.5-, 37-, 55.6-km) radii from each airfield. Each CG lightning strike is binned at 1-, 3-, and 6-hour intervals at each specified radius. The software merges the CG lightning strike time intervals and distance with each wind flow regime and creates probability statistics for each time interval, radii, and flow regime, and stratifies them by month and warm season. The AMU also updated the graphical user interface (GUI) with the new data.

  3. Higher climatological temperature sensitivity of soil carbon in cold than warm climates

    NASA Astrophysics Data System (ADS)

    Koven, Charles D.; Hugelius, Gustaf; Lawrence, David M.; Wieder, William R.

    2017-11-01

    The projected loss of soil carbon to the atmosphere resulting from climate change is a potentially large but highly uncertain feedback to warming. The magnitude of this feedback is poorly constrained by observations and theory, and is disparately represented in Earth system models (ESMs). To assess the climatological temperature sensitivity of soil carbon, we calculate apparent soil carbon turnover times that reflect long-term and broad-scale rates of decomposition. Here, we show that the climatological temperature control on carbon turnover in the top metre of global soils is more sensitive in cold climates than in warm climates and argue that it is critical to capture this emergent ecosystem property in global-scale models. We present a simplified model that explains the observed high cold-climate sensitivity using only the physical scaling of soil freeze-thaw state across climate gradients. Current ESMs fail to capture this pattern, except in an ESM that explicitly resolves vertical gradients in soil climate and carbon turnover. An observed weak tropical temperature sensitivity emerges in a different model that explicitly resolves mineralogical control on decomposition. These results support projections of strong carbon-climate feedbacks from northern soils and demonstrate a method for ESMs to capture this emergent behaviour.

  4. Impact of aerosol vertical distribution on aerosol direct radiative effect and heating rate in the Mediterranean region

    NASA Astrophysics Data System (ADS)

    Pappas, Vasileios; Hatzianastassiou, Nikolaos; Matsoukas, Christos; Koras Carracca, Mario; Kinne, Stefan; Vardavas, Ilias

    2015-04-01

    It is now well-established that aerosols cause an overall cooling effect at the surface and a warming effect within the atmosphere. At the top of the atmosphere (TOA), both positive and negative forcing can be found, depending on a number of other factors, such as surface albedo and relative position of clouds and aerosols. Whilst aerosol surface cooling is important due to its relation with surface temperature and other bio-environmental reasons, atmospheric heating is of special interest as well having significant impacts on atmospheric dynamics, such as formation of clouds and subsequent precipitation. The actual position of aerosols and their altitude relative to clouds is of major importance as certain types of aerosol, such as black carbon (BC) above clouds can have a significant impact on planetary albedo. The vertical distribution of aerosols and clouds has recently drawn the attention of the aerosol community, because partially can account for the differences between simulated aerosol radiative forcing with various models, and therefore decrease the level of our uncertainty regarding aerosol forcing, which is one of our priorities set by IPCC. The vertical profiles of aerosol optical and physical properties have been studied by various research groups around the world, following different methodologies and using various indices in order to present the impact of aerosols on radiation on different altitudes above the surface. However, there is still variability between the published results as to the actual effect of aerosols on shortwave radiation and on heating rate within the atmosphere. This study uses vertical information on aerosols from the Max Planck Aerosol Climatology (MAC-v1) global dataset, which is a combination of model output with quality ground-based measurements, in order to provide useful insight into the vertical profile of atmospheric heating for the Mediterranean region. MAC-v1 and the science behind this aerosol dataset have already

  5. What is the impact of natural variability and aerosol-cloud interaction on the effective radiative forcing of anthropogenic aerosol?

    NASA Astrophysics Data System (ADS)

    Fiedler, S.; Stevens, B.; Mauritsen, T.

    2017-12-01

    comprehensive aerosol-climate models in the framework of the EU-funded project BACCHUS. In the future, MACv2-SP will be used in models participating in the Radiative Forcing Model Intercomparison Project (Pincus et al., 2016).

  6. Modeling Study of the Effect of Anthropogenic Aerosols on Late Spring Drought in South China

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hu, Ning; Liu, Xiaohong

    2013-10-01

    In this study, the mechanisms underlying the decadal variability of late spring precipitation in south China are investigated using the latest version 1 of Community Earth System Model (CESM1). We aim to unravel the effects of different climate forcing agents, such as aerosols and greenhouse gases (GHGs), on the decadal variation of precipitation with transient experiments from pre-industry (for year 1850) to present-day (for year 2000). Our results reveal that: (1) CESM1 can reproduce the climatological features of atmospheric circulation and precipitation for the late spring in south China; (2) Only simulations including the forcing of anthropogenic aerosols can reproducemore » the observed decreasing trend of late spring precipitation from 1950-2000 in south China; (3) Aerosols affect the decadal change of precipitation mainly by altering the large scale atmospheric circulation, and to a less extent by increasing the lower-tropospheric stability to inhibit the convective precipitation; and (4) In comparison, other climate forcing agents, such as GHGs, have much smaller effects on the decadal change of spring precipitation in south China. Key words: precipitation, aerosols, climate change, south China, Community Earth System Model« less

  7. The PSI Artist Project: Aerosol Retention and Accident Management Issues Following a Steam Generator Tube Rupture

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Guntay, Salih; Dehbi, Abdel; Suckow, Detlef

    2002-07-01

    Steam generator tube rupture (SGTR) incidents, such as those, which occurred in various operating pressurized, water reactors in the past, are serious operational concerns and remain among the most risk-dominant events. Although considerable efforts have been spent to understand tube degradation processes, develop improved modes of operation, and take preventative and corrective measures, SGTR incidents cannot be completely ruled out. Under certain conditions, high releases of radionuclides to the environment are possible during design basis accidents (DBA) and severe accidents. The severe accident codes' models for aerosol retention in the secondary side of a steam generator (SG) have not beenmore » assessed against any experimental data, which means that the uncertainties in the source term following an un-isolated SGTR concurrent with a severe accident are not currently quantified. The accident management (AM) procedures aim at avoiding or minimizing the release of fission products from the SG. The enhanced retention of activity within the SG defines the effectiveness of the accident management actions for the specific hardware characteristics and accident conditions of concern. A sound database on aerosol retention due to natural processes in the SG is not available, nor is an assessment of the effect of management actions on these processes. Hence, the effectiveness of the AM in SGTR events is not presently known. To help reduce uncertainties relating to SGTR issues, an experimental project, ARTIST (Aerosol Trapping In a Steam generator), has been initiated at the Paul Scherrer Institut to address aerosol and droplet retention in the various parts of the SG. The test section is comprised of a scaled-down tube bundle, a full-size separator and a full-size dryer unit. The project will study phenomena at the separate effect and integral levels and address AM issues in seven distinct phases: Aerosol retention in 1) the broken tube under dry secondary side

  8. Impact of volcanic aerosols on stratospheric ozone recovery

    NASA Astrophysics Data System (ADS)

    Naik, Vaishali; Horowitz, Larry W.; Daniel Schwarzkopf, M.; Lin, Meiyun

    2017-09-01

    We use transient GFDL-CM3 chemistry-climate model simulations over the 2006-2100 period to show how the influence of volcanic aerosols on the extent and timing of ozone recovery varies with (a) future greenhouse gas scenarios (Representative Concentration Pathway (RCP)4.5 and RCP8.5) and (b) halogen loading. Current understanding is that elevated volcanic aerosols reduce ozone under high halogen loading but increase ozone under low halogen loading when the chemistry is more NOx dominated. With extremely low aerosol loadings (designated here as "background"), global stratospheric ozone burden is simulated to return to 1980 levels around 2050 in the RCP8.5 scenario but remains below 1980 levels throughout the 21st century in the RCP4.5 scenario. In contrast, with elevated volcanic aerosols, ozone column recovers more quickly to 1980 levels, with recovery dates ranging from the mid-2040s in RCP8.5 to the mid-2050s to early 2070s in RCP4.5. The ozone response in both future emission scenarios increases with enhanced volcanic aerosols. By 2100, the 1980 baseline-adjusted global stratospheric ozone column is projected to be 20-40% greater in RCP8.5 and 110-200% greater in RCP4.5 with elevated volcanic aerosols compared to simulations with the extremely low background aerosols. The weaker ozone enhancement at 2100 in RCP8.5 than in RCP4.5 in response to elevated volcanic aerosols is due to a factor of 2.5 greater methane in RCP8.5 compared with RCP4.5. Our results demonstrate the substantial uncertainties in stratospheric ozone projections and expected recovery dates induced by volcanic aerosol perturbations that need to be considered in future model ozone projections.

  9. Peer-tutoring educational experiences about meteorological and climatological issues in Friuli Venezia Giulia (Italy)

    NASA Astrophysics Data System (ADS)

    Nordio, Sergio; Flapp, Federica

    2017-04-01

    The aim of this work is to present some experiences of intergenerational education about meteorology and climatology issues carried out with school pupils from 6 to 19 years old, through peer-tutoring methodology. These experiences started in 2003 and each year the project involves about 500 students in Friuli Venezia Giulia region (about 8.000 km2) in northeastern Italy. A group of volunteers (older students from upper secondary school, 17-19 years old) play the role of "tutor": they receive supplementary training on meteorology and climatology, and then, during students' meetings and/or public events, they teach younger pupils how to use meteorological instruments (thermometer, hygrometer, barometer, anemometer, rain gages, etc.) and they carry out interactive experiences such as "game-experiments", to better understand some meteorological concepts, like density of fluids, and some climatological notions, like the effects of climate change with an exhibit that simulates the greenhouse effect. They also do some meteorological forecasting exercises, using meteorological maps, as if they were actual forecasters. All these activities are addressed to pupils from primary (age 6-11) and lower secondary schools (age 11-14), and both tutors and their younger "apprentices" are not only cognitively, but also emotionally involved in such learning experiences. As a second step of this educational process, after consolidating the above mentioned peer-tutoring activities, high school students hare being actively involved in developing visual tools - e.g. video-clips, interviews and cartoons - in order to communicate climate change issues in the most effective way to younger pupils. Keywords: meteorology, climatology, climate change, schools, education, communication.

  10. Influence of Aerosol Heating on the Stratospheric Transport of the Mt. Pinatubo Eruption

    NASA Technical Reports Server (NTRS)

    Aquila, Valentina; Oman, Luke D.; Stolarski, Richard S.

    2011-01-01

    On June 15th, 1991 the eruption of Mt. Pinatubo (15.1 deg. N, 120.3 Deg. E) in the Philippines injected about 20 Tg of sulfur dioxide in the stratosphere, which was transformed into sulfuric acid aerosol. The large perturbation of the background aerosol caused an increase in temperature in the lower stratosphere of 2-3 K. Even though stratospheric winds climatological]y tend to hinder the air mixing between the two hemispheres, observations have shown that a large part of the SO2 emitted by Mt. Pinatubo have been transported from the Northern to the Southern Hemisphere. We simulate the eruption of Mt. Pinatubo with the Goddard Earth Observing System (GEOS) version 5 global climate model, coupled to the aerosol module GOCART and the stratospheric chemistry module StratChem, to investigate the influence of the eruption of Mt. Pinatubo on the stratospheric transport pattern. We perform two ensembles of simulations: the first ensemble consists of runs without coupling between aerosol and radiation. In these simulations the plume of aerosols is treated as a passive tracer and the atmosphere is unperturbed. In the second ensemble of simulations aerosols and radiation are coupled. We show that the set of runs with interactive aerosol produces a larger cross-equatorial transport of the Pinatubo cloud. In our simulations the local heating perturbation caused by the sudden injection of volcanic aerosol changes the pattern of the stratospheric winds causing more intrusion of air from the Northern into the Southern Hemisphere. Furthermore, we perform simulations changing the injection height of the cloud, and study the transport of the plume resulting from the different scenarios. Comparisons of model results with SAGE II and AVHRR satellite observations will be shown.

  11. Aerosol, cloud, and precipitation interactions in Eastern North Atlantic

    NASA Astrophysics Data System (ADS)

    Wang, J.; Wood, R.; Dong, X.

    2017-12-01

    With their extensive coverage, marine low clouds greatly impact global climate. Presently, marine low clouds are poorly represented in global climate models, and the response of marine low clouds to changes in atmospheric greenhouse gases and aerosols remains the major source of uncertainty in climate simulations. The Eastern North Atlantic (ENA) is a region of persistent but diverse subtropical marine boundary layer clouds, whose albedo and precipitation are highly susceptible to perturbations in aerosol properties. In addition, ENA is periodically impacted by anthropogenic aerosol both from North American and from continental Europe, making it an excellent location to study the CCN budget in a remote marine region periodically perturbed by anthropogenic emissions, and to investigate the impacts of long-range transport of aerosols on remote marine clouds. Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA), funded by DOE Atmospheric Radiation Measurement (ARM) program, is designed to improve the understanding of marine boundary CCN budget, cloud and drizzle microphysics, and the impact of aerosol on marine low cloud and precipitation in the ENA by combining airborne observations and long term surface based measurements. The study has two airborne deployments. The first deployment took place from June 15 to July 25, 2017, and the second one will take place from January 10 to February 20, 2018. Flights during the first deployment were carried out in the Azores, near the ARM ENA site on Graciosa Island. The long term measurements at the ENA site provide important Climatological context for the airborne observations during the two deployments, and the cloud structures provided by the scanning radars at the ENA site put the detailed in-situ measurements into mesoscale and cloud lifecycle contexts. Another important aspect of this study is to provide high quality in-situ measurements for validating and improving ground-based retrieval algorithms at the ENA

  12. Aerosol measurements over the Pacific Ocean in support of the IR aerosol backscatter program

    NASA Technical Reports Server (NTRS)

    Prospero, Joseph M.; Savoie, Dennis L.

    1995-01-01

    The major efforts under NASA contract NAG8-841 included: (1) final analyses of the samples collected during the first GLOBE survey flight that occurred in November 1989 and collections and analysis of aerosol samples during the second GLOBE survey flight in May and June 1990. During the first GLOBE survey flight, daily samples were collected at four stations (Midway, Rarotonga, American Samoa, and Norfolk Island) throughout the month of November 1989. Weekly samples were collected at Shemya, Alaska, and at Karamea, New Zealand. During the second GLOBE survey flight, daily samples were collected at Midway, Oahu, American Samoa, Rarotonga, and Norfolk Island; weekly samples were collected at Shemya. These samples were all analyzed for sodium (sea-salt), chloride, nitrate, sulfate, and methanesulfonate at the University of Miami and for aluminum at the University of Rhode Island (under a subcontract). (2) Samples continued to be collected on a weekly basis at all stations during the periods between and after the survey flights. These weekly samples were also analyzed at the University of Miami for the suite of water-soluble species. (3) In August 1990, the results obtained from the above studies were submitted to the appropriate personnel at NASA Marshall Space Flight Center to become part of the GLOBE data base for comparison with data from instruments used aboard the aircraft. In addition, the data will be compared with data previously obtained at these stations as part of the Sea-Air Exchange (SEAREX) Program. This comparison will provide valuable information on the representativeness of the periods in terms of the longer term aerosol climatology over the Pacific Ocean. (4) Several publications have been written using data from this grant. The data will continue to be used in the future as part of a continuing investigation of the long-term trends and interannual variations in aerosol species concentrations over the Pacific Ocean.

  13. The statistical distribution of aerosol properties in sourthern West Africa

    NASA Astrophysics Data System (ADS)

    Haslett, Sophie; Taylor, Jonathan; Flynn, Michael; Bower, Keith; Dorsey, James; Crawford, Ian; Brito, Joel; Denjean, Cyrielle; Bourrianne, Thierry; Burnet, Frederic; Batenburg, Anneke; Schulz, Christiane; Schneider, Johannes; Borrmann, Stephan; Sauer, Daniel; Duplissy, Jonathan; Lee, James; Vaughan, Adam; Coe, Hugh

    2017-04-01

    The population and economy in southern West Africa have been growing at an exceptional rate in recent years and this trend is expected to continue, with the population projected to more than double to 800 million by 2050. This will result in a dramatic increase in anthropogenic pollutants, already estimated to have tripled between 1950 and 2000 (Lamarque et al., 2010). It is known that aerosols can modify the radiative properties of clouds. As such, the entrainment of anthropogenic aerosol into the large banks of clouds forming during the onset of the West African Monsoon could have a substantial impact on the region's response to climate change. Such projections, however, are greatly limited by the scarcity of observations in this part of the world. As part of the Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa (DACCIWA) project, three research aircraft were deployed, each carrying equipment capable of measuring aerosol properties in-situ. Instrumentation included Aerosol Mass Spectrometers (AMS), Single Particle Soot Photometers (SP2), Condensation Particle Counters (CPC) and Scanning Mobility Particle Sizers (SMPS). Throughout the intensive aircraft campaign, 155 hours of scientific flights covered an area including large parts of Benin, Togo, Ghana and parts of Côte D'Ivoire. Approximately 70 hours were dedicated to the measurement of cloud-aerosol interactions, with many other flights producing data contributing towards this objective. Using datasets collected during this campaign period, it is possible to build a robust statistical understanding of aerosol properties in this region for the first time, including size distributions and optical and chemical properties. Here, we describe preliminary results from aerosol measurements on board the three aircraft. These have been used to describe aerosol properties throughout the region and time period encompassed by the DACCIWA aircraft campaign. Such statistics will be invaluable for improving future

  14. Antarctic Meteorology and Climatology

    NASA Astrophysics Data System (ADS)

    King, J. C.; Turner, J.

    1997-07-01

    This book is a comprehensive survey of the climatology and meteorology of Antarctica. The first section of the book reviews the methods by which we can observe the Antarctic atmosphere and presents a synthesis of climatological measurements. In the second section, the authors consider the processes that maintain the observed climate, from large-scale atmospheric circulation to small-scale processes. The final section reviews our current knowledge of the variability of Antarctic climate and the possible effects of "greenhouse" warming. The authors stress links among the Antarctic atmosphere, other elements of the Antarctic climate system (oceans, sea ice and ice sheets), and the global climate system. This volume will be of greatest interest to meteorologists and climatologists with a specialized interest in Antarctica, but it will also appeal to researchers in Antarctic glaciology, oceanography and biology. Graduates and undergraduates studying physical geography, and the earth, atmospheric and environmental sciences will find much useful background material in the book.

  15. A climatological description of the Savannah River Site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hunter, C.H.

    1990-05-22

    This report provides a general climatological description of the Savannah River Site. The description provides both regional and local scale climatology. The regional climatology includes a general regional climatic description and presents information on occurrence frequencies of the severe meteorological phenomena that are important considerations in the design and siting of a facility. These phenomena include tornadoes, thunderstorms, hurricanes, and ice/snow storms. Occurrence probabilities given for extreme tornado and non-tornado winds are based on previous site specific studies. Local climatological conditions that are significant with respect to the impact of facility operations on the environment are described using on-site ormore » near-site meteorological data. Summaries of wind speed, wind direction, and atmospheric stability are primarily based on the most recently generated five-year set of data collected from the onsite meteorological tower network (1982--86). Temperature, humidity, and precipitation summaries include data from SRL's standard meteorological instrument shelter and the Augusta National Weather Service office at Bush Field through 1986. A brief description of the onsite meteorological monitoring program is also provided. 24 refs., 15 figs., 22 tabs.« less

  16. Role of Climate Change in Global Predictions of Future Tropospheric Ozone and Aerosols

    NASA Technical Reports Server (NTRS)

    Liao, Hong; Chen, Wei-Ting; Seinfeld, John H.

    2006-01-01

    A unified tropospheric chemistry-aerosol model within the Goddard Institute for Space Studies general circulation model II is applied to simulate an equilibrium CO2-forced climate in the year 2100 to examine the effects of climate change on global distributions of tropospheric ozone and sulfate, nitrate, ammonium, black carbon, primary organic carbon, secondary organic carbon, sea salt, and mineral dust aerosols. The year 2100 CO2 concentration as well as the anthropogenic emissions of ozone precursors and aerosols/aerosol precursors are based on the Intergovernmental Panel on Climate Change Special Report on Emissions Scenarios (SRES) A2. Year 2100 global O3 and aerosol burdens predicted with changes in both climate and emissions are generally 5-20% lower than those simulated with changes in emissions alone; as exceptions, the nitrate burden is 38% lower, and the secondary organic aerosol burden is 17% higher. Although the CO2-driven climate change alone is predicted to reduce the global O3 concentrations over or near populated and biomass burning areas because of slower transport, enhanced biogenic hydrocarbon emissions, decomposition of peroxyacetyl nitrate at higher temperatures, and the increase of O3 production by increased water vapor at high NOx levels. The warmer climate influences aerosol burdens by increasing aerosol wet deposition, altering climate-sensitive emissions, and shifting aerosol thermodynamic equilibrium. Climate change affects the estimates of the year 2100 direct radiative forcing as a result of the climate-induced changes in burdens and different climatological conditions; with full gas-aerosol coupling and accounting for ozone and direct radiative forcings by the O2, sulfate, nitrate, black carbon, and organic carbon are predicted to be +0.93, -0.72, -1.0, +1.26, and -0.56 W m(exp -2), respectively, using present-day climate and year 2100 emissions, while they are predicted to be +0.76, -0.72, 0.74, +0.97, and -0.58 W m(exp -2

  17. The Global Precipitation Climatology Project (GPCP): Results, Status and Future

    NASA Technical Reports Server (NTRS)

    Adler, Robert F.

    2007-01-01

    The Global Precipitation Climatology Project (GPCP) is one of a number of long-term, satellite-based, global analyses routinely produced under the auspices of the World Climate Research Program (WCRP) and its Global Energy and Watercycle EXperiment (GEWEX) program. The research quality analyses are produced a few months after real-time through the efforts of scientists at various national agencies and universities in the U.S., Europe and Japan. The primary product is a monthly analysis of surface precipitation that is globally complete and spans the period 1979-present. There are also pentad analyses for the same period and a daily analysis for the 1997-present period. Although generated with somewhat different data sets and analysis schemes, the pentad and daily data sets are forced to agree with the primary monthly analysis on a grid box by grid box basis. The primary input data sets are from low-orbit passive microwave observations, geostationary infrared observations and surface raingauge information. Examples of research with the data sets are discussed, focusing on tropical (25N-25s) rainfall variations and possible long-term changes in the 28-year (1979-2006) monthly dataset. Techniques are used to discriminate among the variations due to ENSO, volcanic events and possible long-term changes for rainfall over both land and ocean. The impact of the two major volcanic eruptions over the past 25 years is estimated to be about a 5% maximum reduction in tropical rainfall during each event. Although the global change of precipitation in the data set is near zero, a small upward linear change over tropical ocean (0.06 mm/day/l0yr) and a slight downward linear change over tropical land (-0.03 mm/day/l0yr) are examined to understand the impact of the inhomogeneity in the data record and the length of the data set. These positive changes correspond to about a 5% increase (ocean) and 3% increase (ocean plus land) during this time period. Relations between variations in

  18. Systematic Differences between Satellite-Based Presipitation Climatologies over the Tropical Oceans

    NASA Technical Reports Server (NTRS)

    Robertson, Frankin R.; Fitzjarrald, Dan; McCaul, Eugene W.

    1999-01-01

    Since the beginning of the World Climate Research Program's Global Precipitation Climatology Project (GPCP) satellite remote sensing of precipitation has made dramatic improvements, particularly for tropical regions. Data from microwave and infrared sensors now form the most critical input to precipitation data sets and can be calibrated with surface gauges to so that the strengths of each data source can be maximized in some statistically optimal sense. It is clear however that there still remain significant uncertainties with satellite precipitation retrievals which limit their usefulness for many purposes. Systematic differences i'A tropical precipitation estimates have been brought to light in comparison activities such as the GPCP Algorithm Intercomparison Project and more recent Wetnet Precipitation Intercomparison Project 3. These uncertainties are assuming more importance because of the demands for validation associated with global climate modeling and data assimilation methodologies. The objective of the present study is to determine the physical basis for systematic differences in spatial structure of tropical precipitation as portrayed by several different satellite-based data sets. The study is limited to oceanic regions only and deals primarily with aspects of spatial variability. We are specifically interested in why MSU channel 1 and GPI precipitation differences are so striking over the Eastern Pacific ITCZ and why they both differ from other microwave emission-based precipitation estimates from SSM/I and a scattering-based deep convective ice index from MSU channel 2. Our results to date have shown that MSU channel I precipitation estimates are biased high over the Eastern Pacific ITCZ because of two factors: (1) the hypersensitivity of this frequency to cloud water in contrast to falling rain drops, and (2) unaccounted for scattering effects by precipitation-size ice which depresses the signal of the liquid water emission. Likewise, cold cloud top

  19. Instrumentation for Aerosol and Gas Speciation

    NASA Technical Reports Server (NTRS)

    Coggiola, Michael J.

    1998-01-01

    Using support from NASA Grant No. NAG 2-963, SRI International successfully completed the project, entitled, 'Instrumentation for Aerosol and Gas Speciation.' This effort (SRI Project 7383) covered the design, fabrication, testing, and deployment of a real-time aerosol speciation instrument in NASA's DC-8 aircraft during the Spring 1996 SUbsonic aircraft: Contrail and Cloud Effects Special Study (SUCCESS) mission. This final technical report describes the pertinent details of the instrument design, its abilities, its deployment during SUCCESS and the data acquired from the mission, and the post-mission calibration, data reduction, and analysis.

  20. The DACCIWA project: Dynamics-aerosol-chemistry-cloud interactions in West Africa

    NASA Astrophysics Data System (ADS)

    Knippertz, Peter

    2017-04-01

    This contribution provides an overview of the EU-funded DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa) project. DACCIWA consists of 16 European and African research organisations and has strong links to universities, weather services and government organisations across West Africa. The project runs from 2010 to 2018 and is built around a major international field campaign in 2016. A key motivation for DACCIWA is the expected tripling of anthropogenic emissions in southern West Africa (SWA) between 2000 and 2030, whose impacts on human health, ecosystems, food security and the regional climate are largely unknown. An integrated assessment of this problem, which is mostly due to massive economic and population growth and urbanization, is challenging due to (a) a superposition of regional effects with global climate change, (b) a strong dependence on the variable West African monsoon, (c) incomplete scientific understanding of interactions between emissions, clouds, radiation, precipitation and regional circulations, and (d) a lack of observations. DACCIWA combines measurements in the field in SWA with extensive modelling activities and work on satellite data. In particular during the main DACCIWA field campaign in June-July 2016 high-quality observations of emissions, atmospheric composition and meteorological parameters were sampled. The campaign involved three research aircraft, three ground-based supersites, enhanced radiosonde launches, and intensive measurements at urban sites in Abidjan and Cotonou. These data have already been quality-controlled and will be freely available to the research community through a database at http://baobab.sedoo.fr/DACCIWA/ after the end of the project. The resulting benchmark dataset is currently combined with a wide range of modelling and satellite-based research activities that will ultimately allow (a) an assessment of the roles of relevant physical, chemical and biological processes, (b) an improvement

  1. New capabilities for characterizing smoke and dust aerosol over land using MODIS

    NASA Astrophysics Data System (ADS)

    Levy, R. C.; Remer, L. A.

    2006-12-01

    Smoke and dust aerosol have different chemical, optical and physical properties and both types affect many processes within the climate system. As earth's surface and atmosphere are continuously altered by natural and anthropogenic processes, the emission and presumably the effects of these aerosols are also changing. Thus it is necessary to observe and characterize aerosols on a global and climatic scale. While MODIS has been reporting characteristics of smoke and dust aerosol over land and ocean since shortly after Terra launch, the uncertainties in the over-land retrieval have been larger than expected. To better characterize different aerosol types closer to their source regions with greater accuracy, we have developed a new operational algorithm for retrieving aerosol properties over dark land surfaces from MODIS-observed visible (VIS) and infrared (IR) reflectance. Like earlier versions, this algorithm estimates the total loading (aerosol optical depth-τ) and relative weighting of fine (non-dust) and coarse (dust) -dominated aerosol to the total τ (fine weighting-η) over dark land surfaces. However, the fundamental mathematics and major assumptions have been overhauled. The new algorithm performs simultaneous multi-channel inversion that includes information about coarse aerosol in the IR channels, while assuming a fine-tuned relationship between VIS and IR surface reflectances, that is itself a function of scattering angle and vegetation condition. Finally, the suite of expected aerosol optical models described by the lookup table have been revised to closer resemble the AERONET climatology, including for smoke and dust aerosol. Beginning in April 2006, this algorithm has been used for forward processing and backward re- processing of the entire MODIS dataset observed from both Terra and Aqua. "Collection 5" products were completed for Aqua reprocessing by July 2006 and should be complete for Terra by December 2006. In this study, we used the complete

  2. Evaluation of the MODIS Aerosol Retrievals over Ocean and Land during CLAMS.

    NASA Astrophysics Data System (ADS)

    Levy, R. C.; Remer, L. A.; Martins, J. V.; Kaufman, Y. J.; Plana-Fattori, A.; Redemann, J.; Wenny, B.

    2005-04-01

    climatology for the MODIS lookup table over land, it is shown that the low bias for larger aerosol loadings can also be corrected. Understanding and improving MODIS retrievals over the East Coast may point to strategies for correction in other locations, thus improving the global quality of MODIS. Improvements in regional aerosol detection could also lead to the use of MODIS for monitoring air pollution.

  3. Operational remote sensing of tropospheric aerosol over land from EOS moderate resolution imaging spectroradiometer

    NASA Astrophysics Data System (ADS)

    Kaufman, Y. J.; Tanré, D.; Remer, L. A.; Vermote, E. F.; Chu, A.; Holben, B. N.

    1997-07-01

    sensing from the ground, will be used to study aerosol climatology, to monitor the sources and sinks of specific aerosol types, and to study the interaction of aerosol with water vapor and clouds and their radiative forcing of climate. The aerosol information will also be used for atmospheric corrections of remotely sensed surface reflectance. In this paper, examples of applications and validations are provided.

  4. Radiative Flux Changes by Aerosols from North America, Europe, and Africa over the Atlantic Ocean: Measurements and Calculations from TARFOX and ACE-2

    NASA Technical Reports Server (NTRS)

    Russell, P. B.; Hignett, P.; Livingston, J. M.; Schmid, B.; Chien, A.; Bergstrom, R.; Durkee, P. A.; Hobbs, P. V.; Bates, T. S.; Quinn, P. K.; hide

    1998-01-01

    Aerosol effects on atmospheric radiative fluxes provide a forcing function that is a major source of uncertainty in understanding the past climate and predicting climate change. To help reduce this uncertainty, the 1996 Tropospheric Aerosol Radiative Forcing Experiment (TARFOX) and the 1997 second Aerosol Characterization Experiment (ACE-2) measured the properties and radiative effects of American, European, and African aerosols over the Atlantic. In TARFOX, radiative fluxes and microphysics of the American aerosol were measured from the UK C-130 while optical depth spectra, aerosol composition, and other properties were measured by the University of Washington C-131A and the CIRPAS Pelican. Closure studies show that the measured flux changes agree with those derived from the aerosol measurements using several modelling approaches. The best-fit midvisible single-scatter albedos (approx. 0.89 to 0.93) obtained from the TARFOX flux comparisons are in accord with values derived by independent techniques. In ACE-2 we measured optical depth and extinction spectra for both European urban-marine aerosols and free-tropospheric African dust aerosols, using sunphotometers on the R/V Vodyanitskiy and the Pelican. Preliminary values for the radiative flux sensitivities (Delta Flux / Delta Optical depth) computed for ACE-2 aerosols (boundary layer and African dust) over ocean are similar to those found in TARFOX. Combining a satellite-derived optical depth climatology with the aerosol optical model validated for flux sensitivities in TARFOX provides first-cut estimates of aerosol-induced flux changes over the Atlantic Ocean.

  5. Characterization of the Aerosol Instrument Package for the In-service Aircraft Global Observing System IAGOS

    NASA Astrophysics Data System (ADS)

    Bundke, Ulrich; Berg, Marcel; Tettig, Frank; Franke, Harald; Petzold, Andreas

    2015-04-01

    The atmospheric aerosol influences the climate twofold via the direct interaction with solar radiation and indirectly effecting microphysical properties of clouds. The latter has the largest uncertainty according to the last IPPC Report. A measured in situ climatology of the aerosol microphysical properties is needed to reduce the reported uncertainty of the aerosol climate impact. The European Research Infrastructure IAGOS (In-service Aircraft for a Global Observing System; www.iagos.org) responds to the increasing requests for long-term, routine in situ observational data by using commercial passenger aircraft as measurement platform. However, scientific instrumentation for the measurement of atmospheric constituents requires major modifications before being deployable aboard in-service passenger aircraft. The IAGOS Aerosol Package (IAGOS-P2C) consists of two modified Butanol based CPCs (Model Grimm 5.410) and one optical particle counter (Model Grimm Sky OPC 1.129). A thermodenuder at 250°C is placed upstream the second CPC, thus the number concentrations of the total aerosol and the non-volatile aerosol fraction is measured. The Sky OPC measures the size distribution in the rage theoretically up to 32 μ m. Because of the inlet cut off diameter of D50=3 μ m we are using the 16 channel mode in the range of 250 nm - 2.5 μ m at 1 Hz resolution. In this presentation the IAGOS Aerosol package is characterized for pressure levels relevant for the planned application, down to cruising level of 150 hPa including the inlet system. In our aerosol lab we have tested the system against standard instrumentation with different aerosol test substances in a long duration test. Particle losses are characterized for the inlet system. In addition first results for airborne measurements are shown from a first field campaign.

  6. Aerosol optical properties and direct radiative forcing based on measurements from the China Aerosol Remote Sensing Network (CARSNET) in eastern China

    NASA Astrophysics Data System (ADS)

    Che, Huizheng; Qi, Bing; Zhao, Hujia; Xia, Xiangao; Eck, Thomas F.; Goloub, Philippe; Dubovik, Oleg; Estelles, Victor; Cuevas-Agulló, Emilio; Blarel, Luc; Wu, Yunfei; Zhu, Jun; Du, Rongguang; Wang, Yaqiang; Wang, Hong; Gui, Ke; Yu, Jie; Zheng, Yu; Sun, Tianze; Chen, Quanliang; Shi, Guangyu; Zhang, Xiaoye

    2018-01-01

    Aerosol pollution in eastern China is an unfortunate consequence of the region's rapid economic and industrial growth. Here, sun photometer measurements from seven sites in the Yangtze River Delta (YRD) from 2011 to 2015 were used to characterize the climatology of aerosol microphysical and optical properties, calculate direct aerosol radiative forcing (DARF) and classify the aerosols based on size and absorption. Bimodal size distributions were found throughout the year, but larger volumes and effective radii of fine-mode particles occurred in June and September due to hygroscopic growth and/or cloud processing. Increases in the fine-mode particles in June and September caused AOD440 nm > 1.00 at most sites, and annual mean AOD440 nm values of 0.71-0.76 were found at the urban sites and 0.68 at the rural site. Unlike northern China, the AOD440 nm was lower in July and August (˜ 0.40-0.60) than in January and February (0.71-0.89) due to particle dispersion associated with subtropical anticyclones in summer. Low volumes and large bandwidths of both fine-mode and coarse-mode aerosol size distributions occurred in July and August because of biomass burning. Single-scattering albedos at 440 nm (SSA440 nm) from 0.91 to 0.94 indicated particles with relatively strong to moderate absorption. Strongly absorbing particles from biomass burning with a significant SSA wavelength dependence were found in July and August at most sites, while coarse particles in March to May were mineral dust. Absorbing aerosols were distributed more or less homogeneously throughout the region with absorption aerosol optical depths at 440 nm ˜ 0.04-0.06, but inter-site differences in the absorption Angström exponent indicate a degree of spatial heterogeneity in particle composition. The annual mean DARF was -93 ± 44 to -79 ± 39 W m-2 at the Earth's surface and ˜ -40 W m-2 at the top of the atmosphere (for the solar zenith angle range of 50 to 80°) under cloud-free conditions. The fine mode

  7. Study of the consistency of climatological products of Nimbus-7

    NASA Technical Reports Server (NTRS)

    Dhuria, Harbans L.

    1988-01-01

    The study, in addition to investigating the consistency of climatological products from Nimbus-7 Earth Radiation Budget and Temperature Humidity Infrared Radiometer experiments, focussed on the climatological analysis of the specified regions of the Earth. The climatological study consisted of the effects of various types of clouds on the net radiation, albedos, and emitted radiation. In addition to a correlational study for determining consistency level of data, a population study of the regions was formulated and conducted. The regions under this study were formed by clustering the target areas using the criteria of climatological conditions such as geography, ocean, and land. Research is limited to tropics from 18 deg north to 18 deg south. A correlational study indicates that there is high positive correlation between high clouds and albedo, and a reduced negative correlation between albedo and net radiation.

  8. A Water Mass Tracer Detected in Aerosols Demonstrates Ocean-Atmosphere Mass Transfer and Links Sea Spray Aerosol to Source Waters

    NASA Astrophysics Data System (ADS)

    Pendergraft, M.; Grimes, D. J.; Giddings, S. N.; Feddersen, F.; Prather, K. A.; Santander, M.; Lee, C.; Beall, C.

    2016-12-01

    During September and October of 2015 the Cross Surfzone/Inner-shelf Dye Exchange (CSIDE) project released rhodamine WT dye to study nearshore water movement and exchange offshore along a Southern California sandy beach. We utilized this opportunity to investigate ocean-atmosphere mass transfer via sea spray aerosol and linkage to source waters. Aerosol-concentrating sampling equipment was deployed at beachside and inland locations during three dye releases. Concentrated aerosol samples were analyzed for dye content using fluorescence spectroscopy. Here we present the ocean and atmosphere conditions associated with the presence and absence of dye in aerosol samples. Dye was identified in aerosol samples collected 0.1-0.3 km from the shoreline for 6 hs during the first and third dye releases of the CSIDE project. During these releases the dye persisted in the waters upwind of the sampling equipment. Dye was not detected in aerosol samples collected during the second release during which dye was moved away from waters upwind of the sampling equipment. Recovery of a chemical tracer in sea spray aerosol allows direct linkage to a known source area in the ocean that is independent of, but supported by, wind data. Our observations demonstrate: a tight ocean-atmosphere spatial coupling; a short residence time of coastal marine constituents before transfer to the atmosphere; that the ocean is both a sink for and a source of atmospheric and terrestrial material; and that human inputs to the ocean can return to us in sea spray aerosol.

  9. Comparison of TRMM and Global Precipitation Climatology Project (GPCP) Precipitation Analyses

    NASA Technical Reports Server (NTRS)

    Adler, Robert F.; Huffman, George J.; Bolvin, David; Nelkin, Eric; Curtis, Scott

    1999-01-01

    This paper describes recent results of using Tropical Rainfall Measuring Mission (TRMM) (launched in November 1997) information as the key calibration tool in a merged analysis on a 1 x 1' latitude/longitude monthly scale based on multiple satellite sources and raingauge analyses. The TRMM-based product is compared with the community-based Global Precipitation Climatology Project (GPCP) results. The long-term GPCP analysis is compared to the new TRMM-based analysis which uses the most accurate TRMM information to calibrate the estimates from the Special Sensor Microwave/Imager (SSM/I) and geosynchronous IR observations and merges those estimates together with the TRMM and gauge information to produce accurate rainfall estimates with the increased sampling provided by the combined satellite information. The comparison with TRMM results on a month-to-month basis should clarify the strengths and weaknesses of the long-term GPCP product in the tropics and point to how to improve the monitoring analysis. Preliminary results from the TRMM merged satellite analysis indicates fairly close agreement with the GPCP estimates. The GPCP analysis is done at 2.5 degree latitude/longitude resolution and interpolated to a 1 degree grid for comparison with the TRMM analysis. As expected the same features are evident in both panels, but there are subtle differences in the magnitudes. Focusing on the Pacific Ocean Inter-Tropical Convergence Zone (ITCZ) one can see the TRMM-based estimates having higher peak values and lower values in the ITCZ periphery. These attributes also show up in the statistics, where GPCP>TRMM at low values (below 10 mm/d) and TRMM>GPCP at high values (greater than 15 mm/d). The area in the Indian Ocean which shows consistently higher values of TRMM over GPCP needs to be examined carefully to determine if the lack of geosynchronous data has led to a difference in the two analyses. By the time of the meeting over a year of TRMM products will be available for

  10. Inter-annual variability of aerosol optical depth over the tropical Atlantic Ocean based on MODIS-Aqua observations over the period 2002-2012

    NASA Astrophysics Data System (ADS)

    Gkikas, Antonis; Hatzianastassiou, Nikolaos

    2013-04-01

    The tropical Atlantic Ocean is affected by dust and biomass burning aerosol loads transported from the western parts of the Saharan desert and the sub-Sahel regions, respectively. The spatial and temporal patterns of this transport are determined by the aerosol emission rates, their deposition (wet and dry), by the latitudinal shift of the Intertropical Convergence Zone (ITCZ) and the prevailing wind fields. More specifically, in summer, Saharan dust aerosols are transported towards the Atlantic Ocean, even reaching the Gulf of Mexico, while in winter the Atlantic Ocean transport takes place in more southern latitudes, near the equator, sometimes reaching the northern parts of South America. In the later case, dust is mixed with biomass burning aerosols originating from agricultural activities in the sub-Sahel, associated with prevailing north-easterly airflow (Harmattan winds). Satellite observations are the appropriate tool for describing this African aerosol export, which is important to atmospheric, oceanic and climate processes, offering the advantage of complete spatial coverage. In the present study, we use satellite measurements of aerosol optical depth at 550nm (AOD550nm), on a daily and monthly basis, derived from MODIS-Aqua platform, at 1ox1o spatial resolution (Level 3), for the period 2002-2012. The primary objective is to determine the pixel-level and regional mean anomalies of AOD550nm over the entire study period. The regime of the anomalies of African export is interpreted in relation to the aerosol source areas, precipitation, wind patterns and temporal variability of the North Atlantic Oscillation Index (NAOI). In order to ensure availability of AOD over the Sahara desert, MODIS-Aqua Deep Blue products are also used. As for precipitation, Global Precipitation Climatology Project (GPCP) data at 2.5ox2.5o are used. The wind fields are taken from the National Center for Environmental Prediction (NCEP). Apart from the regime of African aerosol export

  11. Impact of aerosol emission controls on future Arctic sea ice cover

    NASA Astrophysics Data System (ADS)

    Gagné, M.-Ã..; Gillett, N. P.; Fyfe, J. C.

    2015-10-01

    We examine the response of Arctic sea ice to projected aerosol and aerosol precursor emission changes under the Representative Concentration Pathway (RCP) scenarios in simulations of the Canadian Earth System Model. The overall decrease in aerosol loading causes a warming, largest over the Arctic, which leads to an annual mean reduction in sea ice extent of approximately 1 million km2 over the 21st century in all RCP scenarios. This accounts for approximately 25% of the simulated reduction in sea ice extent in RCP 4.5, and 40% of the reduction in RCP 2.5. In RCP 4.5, the Arctic ocean is projected to become ice-free during summertime in 2045, but it does not become ice-free until 2057 in simulations with aerosol precursor emissions held fixed at 2000 values. Thus, while reductions in aerosol emissions have significant health and environmental benefits, their substantial contribution to projected Arctic climate change should not be overlooked.

  12. Response to "Toward Unified Satellite Climatology of Aerosol Properties. 3. MODIS Versus MISR Versus AERONET"

    NASA Technical Reports Server (NTRS)

    Kahn, Ralph A.; Garay, Michael J.; Nelson, David L.; Levy, Robert C.; Bull, Michael A.; Diner, David J.; Martonchik, John V.; Hansen, Earl G.; Remer, Lorraine A.; Tanre, Didier

    2010-01-01

    A recent paper by Mishchenko et al. compares near-coincident MISR, MODIS, and AERONET aerosol optical depth (AOD) products, and reports much poorer agreement than that obtained by the instrument teams and others. We trace the reasons for the discrepancies primarily to differences in (1) the treatment of outliers, (2) the application of absolute vs. relative criteria for testing agreement, and (3) the ways in which seasonally varying spatial distributions of coincident retrievals are taken into account.

  13. Global Distribution of Aerosols Over the Open Ocean as Derived from the Coastal Zone Color Scanner

    NASA Technical Reports Server (NTRS)

    Stegmann, P. M.; Tindale, N. W.

    1999-01-01

    Climatological maps of monthly mean aerosol radiance levels derived from the coastal zone color scanner (CZCS) were constructed for the world's ocean basins. This is the first study to use the 7.5.-year CZCS data set to examine the distribution and seasonality of aerosols over the open ocean on a global scale. Examination of our satellite images found the most prominent large-scale patch of elevated aerosol radiances in each month off the coast of northwest Africa. The well-known, large-scale plumes of elevated aerosol levels in the Arabian Sea, the northwest Pacific, and off the east coast of North America were also successfully captured. Radiance data were extracted from 13 major open-ocean zones, ranging from the subpolar to equatorial regions. Results from these extractions revealed the aerosol load in both subpolar and subtropical zones to be higher in the Northern Hemisphere than in the Southern Hemisphere. Aerosol radiances in the subtropics of both hemispheres were about 2 times higher in summer than in winter. In subpolar regions, aerosol radiances in late spring/early summer were almost 3 times that observed in winter. In general, the aerosol signal was higher during the warmer months and lower during the cooler months, irrespective of location. A comparison between our mean monthly aerosol radiance maps with mean monthly chlorophyll maps (also from CZCS) showed similar seasonality between aerosol and chlorophyll levels in the subpolar zones of both hemispheres, i.e., high levels in summer, low levels in winter. In the subtropics of both hemispheres, however, chlorophyll levels were higher in winter months which coincided with a depressed aerosol signal. Our results indicate that the near-IR channel on ocean color sensors can be used to successfully capture well-known, large-scale aerosol plumes on a global scale and that future ocean color sensors may provide a platform for long-term synoptic studies of combined aerosol-phytoplankton productivity

  14. Improving Satellite Retrieved Infrared Sea Surface Temperatures in Aerosol-Contaminated Regions

    NASA Astrophysics Data System (ADS)

    Luo, B.; Minnett, P. J.; Szczodrak, G.; Kilpatrick, K. A.

    2017-12-01

    Infrared satellite observations of sea surface temperature (SST) have become essential for many applications in meteorology, climatology, and oceanography. Applications often require high accuracy SST data: for climate research and monitoring an absolute uncertainty of 0.1K and stability of better than 0.04K per decade are required. Tropospheric aerosol concentrations increase infrared signal attenuation and prevent the retrieval of accurate satellite SST. We compare satellite-derived skin SST with measurements from the Marine-Atmospheric Emitted Radiance Interferometer (M-AERI) deployed on ships during the Aerosols and Ocean Science Expeditions (AEROSE) and with quality-controlled drifter temperatures. After match-up with in-situ SST and filtering of cloud contaminated data, the results indicate that SST retrieved from MODIS (Moderate Resolution Imaging Spectroradiometer) aboard the Terra and Aqua satellites have negative (cool) biases compared to shipboard radiometric measurements. There is also a pronounced negative bias in the Saharan outflow area that can introduce SST errors >1 K at aerosol optical depths > 0.5. In this study, we present a new method to derive night-time Saharan Dust Index (SDI) algorithms based on simulated brightness temperatures at infrared wavelengths of 3.9, 10.8 and 12.0 μm, derived using RTTOV. We derived correction coefficients for Aqua MODIS measurements by regression of the SST errors against the SDI. The biases and standard deviations are reduced by 0.25K and 0.19K after the SDI correction. The goal of this study is to understand better the characteristics and physical mechanisms of aerosol effects on satellite retrieved infrared SST, as well as to derive empirical formulae for improved accuracies in aerosol-contaminated regions.

  15. Status and Plans for the WCRP/GEWEX Global Precipitation Climatology Project (GPCP)

    NASA Technical Reports Server (NTRS)

    Adkerm Robert F.

    2006-01-01

    Status and plans for GPCP are presented along with scientific findings from the current data set. Global and large regional rainfall variations and possible long-term changes are examined using the 26-year (1979-2004) monthly dataset from the Global Precipitation Climatology Project (GPCP). One emphasis is to discriminate among the variations due to ENSO, volcanic events and possible long-term changes. Although the global change of precipitation in the data set is near zero, the data set does indicate an upward trend (0.13 mm/day/25yr) and a downward trend (-0.06 mm/day/25yr) over tropical oceans and lands (25S-25N), respectively. This corresponds to a 4% increase (ocean) and 2% decrease (land) during this time period. Simple techniques are derived to attempt to eliminate variations due to ENSO and major volcanic eruptions in the Tropics. Using only annual values two "volcano years" are determined by examining ocean-land coupled variations in precipitation related to ENSO and other phenomena. The outlier years coincide with Pinatubo and El Chicon eruptions. The ENSO signal is reduced by deriving mean ocean and land values for El Nino, La Nina and neutral conditions based on Nino 3.4 SST and normalizing the annual ocean and land precipitation to the neutral set of cases. The impact of the two major volcanic eruptions over the past 25 years is estimated to be about a 5% reduction in tropical rainfall. The modified data set (with ENSO and volcano effect at least partially removed) retains the same approximate linear change slopes over the data set period, but with reduced variance leading to significance tests with results in the 90-95% range. Intercomparisons between the GPCP, SSM/I (1988-2004), and TRMM (1998-2004) satellite rainfall products and alternate gauge analyses over land are made to attempt to increase or decrease confidence in the changes seen in the GPCP analysis.

  16. LIVAS: a 3-D multi-wavelength aerosol/cloud database based on CALIPSO and EARLINET

    NASA Astrophysics Data System (ADS)

    Amiridis, V.; Marinou, E.; Tsekeri, A.; Wandinger, U.; Schwarz, A.; Giannakaki, E.; Mamouri, R.; Kokkalis, P.; Binietoglou, I.; Solomos, S.; Herekakis, T.; Kazadzis, S.; Gerasopoulos, E.; Proestakis, E.; Kottas, M.; Balis, D.; Papayannis, A.; Kontoes, C.; Kourtidis, K.; Papagiannopoulos, N.; Mona, L.; Pappalardo, G.; Le Rille, O.; Ansmann, A.

    2015-07-01

    We present LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies), a 3-D multi-wavelength global aerosol and cloud optical database, optimized to be used for future space-based lidar end-to-end simulations of realistic atmospheric scenarios as well as retrieval algorithm testing activities. The LIVAS database provides averaged profiles of aerosol optical properties for the potential spaceborne laser operating wavelengths of 355, 532, 1064, 1570 and 2050 nm and of cloud optical properties at the wavelength of 532 nm. The global database is based on CALIPSO observations at 532 and 1064 nm and on aerosol-type-dependent backscatter- and extinction-related Ångström exponents, derived from EARLINET (European Aerosol Research Lidar Network) ground-based measurements for the UV and scattering calculations for the IR wavelengths, using a combination of input data from AERONET, suitable aerosol models and recent literature. The required spectral conversions are calculated for each of the CALIPSO aerosol types and are applied to CALIPSO backscatter and extinction data corresponding to the aerosol type retrieved by the CALIPSO aerosol classification scheme. A cloud optical database based on CALIPSO measurements at 532 nm is also provided, neglecting wavelength conversion due to approximately neutral scattering behavior of clouds along the spectral range of LIVAS. Averages of particle linear depolarization ratio profiles at 532 nm are provided as well. Finally, vertical distributions for a set of selected scenes of specific atmospheric phenomena (e.g., dust outbreaks, volcanic eruptions, wild fires, polar stratospheric clouds) are analyzed and spectrally converted so as to be used as case studies for spaceborne lidar performance assessments. The final global data set includes 4-year (1 January 2008-31 December 2011) time-averaged CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) data on a uniform grid of 1

  17. Study of MPLNET-Derived Aerosol Climatology over Kanpur, India, and Validation of CALIPSO Level 2 Version 3 Backscatter and Extinction Products

    NASA Technical Reports Server (NTRS)

    Misra, Amit; Tripathi, S. N.; Kaul, D. S.; Welton, Ellsworth J.

    2012-01-01

    The level 2 aerosol backscatter and extinction profiles from the NASA Micropulse Lidar Network (MPLNET) at Kanpur, India, have been studied from May 2009 to September 2010. Monthly averaged extinction profiles from MPLNET shows high extinction values near the surface during October March. Higher extinction values at altitudes of 24 km are observed from April to June, a period marked by frequent dust episodes. Version 3 level 2 Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) aerosol profile products have been compared with corresponding data from MPLNET over Kanpur for the above-mentioned period. Out of the available backscatter profiles, the16 profiles used in this study have time differences less than 3 h and distances less than 130 km. Among these profiles, four cases show good comparison above 400 m with R2 greater than 0.7. Comparison with AERONET data shows that the aerosol type is properly identified by the CALIOP algorithm. Cloud contamination is a possible source of error in the remaining cases of poor comparison. Another source of error is the improper backscatter-to-extinction ratio, which further affects the accuracy of extinction coefficient retrieval.

  18. Final Project Report - ARM CLASIC CIRPAS Twin Otter Aerosol

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    John A. Ogren

    2010-04-05

    The NOAA/ESRL/GMD aerosol group made three types of contributions related to airborne measurements of aerosol light scattering and absorption for the Cloud and Land Surface Interaction Campaign (CLASIC) in June 2007 on the Twin Otter research airplane operated by the Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS). GMD scientists served as the instrument mentor for the integrating nephelometer and particle soot absorption photometer (PSAP) on the Twin Otter during CLASIC, and were responsible for (1) instrument checks/comparisons; (2) instrument trouble shooting/repair; and (3) data quality control (QC) and submittal to the archive.

  19. Aerosol optical characteristics and their vertical distributions under enhanced haze pollution events: effect of the regional transport of different aerosol types over eastern China

    NASA Astrophysics Data System (ADS)

    Sun, Tianze; Che, Huizheng; Qi, Bing; Wang, Yaqiang; Dong, Yunsheng; Xia, Xiangao; Wang, Hong; Gui, Ke; Zheng, Yu; Zhao, Hujia; Ma, Qianli; Du, Rongguang; Zhang, Xiaoye

    2018-03-01

    The climatological variation of aerosol properties and the planetary boundary layer (PBL) during 2013-2015 over the Yangtze River Delta (YRD) region were investigated by employing ground-based Micro Pulse Lidar (MPL) and CE-318 sun-photometer observations. Combining Moderate Resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite products, enhanced haze pollution events affected by different types of aerosol over the YRD region were analyzed through vertical structures, spatial distributions, backward trajectories, and the potential source contribution function (PSCF) model. The results show that aerosols in the YRD are dominated by fine-mode particles, except in March. The aerosol optical depth (AOD) in June and September is higher due to high single scattering albedo (SSA) from hygroscopic growth, but it is lower in July and August due to wet deposition from precipitation. The PBL height (PBLH) is greater (means ranging from 1.23 to 1.84 km) and more variable in the warmer months of March to August, due to the stronger diurnal cycle and exchange of heat. Northern fine-mode pollutants are brought to the YRD at a height of 1.5 km. The SSA increases, blocking the radiation to the surface, and cooling the surface, thereby weakening turbulence, lowering the PBL, and in turn accelerating the accumulation of pollutants, creating a feedback to the cooling effect. Originated from the deserts in Xinjiang and Inner Mongolia, long-range transported dust masses are seen at heights of about 2 km over the YRD region with an SSA440 nm below 0.84, which heat air and raise the PBL, accelerating the diffusion of dust particles. Regional transport from biomass-burning spots to the south of the YRD region bring mixed aerosol particles at a height below 1.5 km, resulting in an SSA440 nm below 0.89. During the winter, the accumulation of the local emission layer is facilitated by stable weather conditions

  20. Aerosol Optical Depth spatiotemporal variability and contribution of different aerosol types over Eastern Mediterranean

    NASA Astrophysics Data System (ADS)

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos; Zanis, Prodromos; Pöschl, Ulrich; Lelieveld, Jos; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios; Pozzer, Andrea

    2015-04-01

    In this work, we study the aerosol spatiotemporal variability over the region of Eastern Mediterranean, for the time period 2000-2012, using a 0.1-degree gridded dataset compiled from level-2 MODIS TERRA and MODIS AQUA AOD550 and FMR550 data. A detailed validation of the AOD550 data was implemented using ground-based observations from the AERONET, also showing that the gridding methodology we followed allows for the detection of several local hot spots that cannot be seen using lower resolutions or level-3 data. By combining the MODIS data with data from other satellite sensors (TOMS, OMI), data from a global chemical-aerosol-transport model (GOCART), and reanalysis data from MACC and ERA-interim, we quantify the relative contribution of different aerosol types to the total AOD550 for the period of interest. For this reason, we developed an optimized algorithm for regional studies based on results from previous global studies. Over land, anthropogenic, dust, and fine-mode natural aerosols contribute to the total AOD550, while anthropogenic, dust and maritime AODs are calculated over the ocean. The dust AOD550 over the region was compared against dust AODs from the LIVAS CALIPSO product, showing a similar seasonal variability. Finally, we also look into the aerosol load short-term trends over the region for each aerosol type separately, the results being strongly affected by the selected time period. The research leading to these results has received funding from the European Social Fund (ESF) and national resources under the operational programme Education and Lifelong Learning (EdLL) within the framework of the Action "Supporting Postdoctoral Researchers" (QUADIEEMS project) and from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement no. 226144 (C8 project).

  1. Remote Sensing of Aerosol in the Terrestrial Atmosphere from Space: New Missions

    NASA Technical Reports Server (NTRS)

    Milinevsky, G.; Yatskiv, Ya.; Degtyaryov, O.; Syniavskyi, I.; Ivanov, Yu.; Bovchaliuk, A.; Mishchenko, M.; Danylevsky, V.; Sosonkin, M.; Bovchaliuk, V.

    2015-01-01

    The distribution and properties of atmospheric aerosols on a global scale are not well known in terms of determination of their effects on climate. This mostly is due to extreme variability of aerosol concentrations, properties, sources, and types. Aerosol climate impact is comparable to the effect of greenhouse gases, but its influence is more difficult to measure, especially with respect to aerosol microphysical properties and the evaluation of anthropogenic aerosol effect. There are many satellite missions studying aerosol distribution in the terrestrial atmosphere, such as MISR/Terra, OMI/Aura, AVHHR, MODIS/Terra and Aqua, CALIOP/CALIPSO. To improve the quality of data and climate models, and to reduce aerosol climate forcing uncertainties, several new missions are planned. The gap in orbital instruments for studying aerosol microphysics has arisen after the Glory mission failed during launch in 2011. In this review paper, we describe several planned aerosol space missions, including the Ukrainian project Aerosol-UA that obtains data using a multi-channel scanning polarimeter and wide-angle polarimetric camera. The project is designed for remote sensing of the aerosol microphysics and cloud properties on a global scale.

  2. Active Learning in Introductory Climatology.

    ERIC Educational Resources Information Center

    Dewey, Kenneth F.; Meyer, Steven J.

    2000-01-01

    Introduces a software package available for the climatology curriculum that determines possible climatic events according to a long-term climate history. Describes the integration of the software into the curriculum and presents examples of active learning. (Contains 19 references.) (YDS)

  3. An operational retrieval algorithm for determining aerosol optical properties in the ultraviolet

    NASA Astrophysics Data System (ADS)

    Taylor, Thomas E.; L'Ecuyer, Tristan S.; Slusser, James R.; Stephens, Graeme L.; Goering, Christian D.

    2008-02-01

    This paper describes a number of practical considerations concerning the optimization and operational implementation of an algorithm used to characterize the optical properties of aerosols across part of the ultraviolet (UV) spectrum. The algorithm estimates values of aerosol optical depth (AOD) and aerosol single scattering albedo (SSA) at seven wavelengths in the UV, as well as total column ozone (TOC) and wavelength-independent asymmetry factor (g) using direct and diffuse irradiances measured with a UV multifilter rotating shadowband radiometer (UV-MFRSR). A novel method for cloud screening the irradiance data set is introduced, as well as several improvements and optimizations to the retrieval scheme which yield a more realistic physical model for the inversion and increase the efficiency of the algorithm. Introduction of a wavelength-dependent retrieval error budget generated from rigorous forward model analysis as well as broadened covariances on the a priori values of AOD, SSA and g and tightened covariances of TOC allows sufficient retrieval sensitivity and resolution to obtain unique solutions of aerosol optical properties as demonstrated by synthetic retrievals. Analysis of a cloud screened data set (May 2003) from Panther Junction, Texas, demonstrates that the algorithm produces realistic values of the optical properties that compare favorably with pseudo-independent methods for AOD, TOC and calculated Ångstrom exponents. Retrieval errors of all parameters (except TOC) are shown to be negatively correlated to AOD, while the Shannon information content is positively correlated, indicating that retrieval skill improves with increasing atmospheric turbidity. When implemented operationally on more than thirty instruments in the Ultraviolet Monitoring and Research Program's (UVMRP) network, this retrieval algorithm will provide a comprehensive and internally consistent climatology of ground-based aerosol properties in the UV spectral range that can be used

  4. A Radar Climatology for Germany - a 16-year high resolution precipitation data and its possibilities

    NASA Astrophysics Data System (ADS)

    Walawender, Ewelina; Winterrath, Tanja; Brendel, Christoph; Hafer, Mario; Junghänel, Thomas; Klameth, Anna; Weigl, Elmar; Becker, Andreas

    2017-04-01

    One of the main features of heavy precipitation events is their small-scale distribution. Despite a local occurrence, these intensive rainfalls may, however, cause most serious damage and have significant impact on the whole river basin area resulting in e.g. flash floods or urban flooding. Thus, it is of great importance not only to detect the life-cycle of extreme precipitation during its occurrence but also to collect precise climatological information on such events. The German weather service (Deutscher Wetterdienst) operates a very dense network of more than 2000 weather stations collecting data on precipitation. It is however not sufficient for detecting spatially limited phenomena. Thanks to radar data, current monitoring of such events is possible. A quality control process is applied to real-time radar products, however only automatic rain gauges data can be used in the adjustment procedure. To merge both radar data and all available rain gauges data, the radar climatology dataset was established. Within the framework of a project financed by the federal agencies' strategic alliance 'Adaptation to Climate Change', 16 years (2001-2016) of radar data have been reanalyzed in order to gain a homogenous, quality-controlled, high-resolution precipitation data set suitable for analyzing extreme events in a climatological approach. Additional corrections methods (e.g. clutter, spokes and beam height correction) were defined and used for the reprocessing procedure to enhance the data quality. Although the time series is still rather short for a climatology, for the first time the data set allows an insight into e.g. the distribution, size, life cycle, and duration of extreme events that cannot be measured by point measurements alone. All radar climatology products share the same spatial and temporal coverage. The whole dataset has been produced for the area of Germany. With the relatively high spatial resolution of 1km, the data can be used as a component of wide

  5. Eight Year Climatologies from Observational (AIRS) and Model (MERRA) Data

    NASA Technical Reports Server (NTRS)

    Hearty, Thomas; Savtchenko, Andrey; Won, Young-In; Theobalk, Mike; Vollmer, Bruce; Manning, Evan; Smith, Peter; Ostrenga, Dana; Leptoukh, Greg

    2010-01-01

    We examine climatologies derived from eight years of temperature, water vapor, cloud, and trace gas observations made by the Atmospheric Infrared Sounder (AIRS) instrument flying on the Aqua satellite and compare them to similar climatologies constructed with data from a global assimilation model, the Modern Era Retrospective-Analysis for Research and Applications (MERRA). We use the AIRS climatologies to examine anomalies and trends in the AIRS data record. Since sampling can be an issue for infrared satellites in low earth orbit, we also use the MERRA data to examine the AIRS sampling biases. By sampling the MERRA data at the AIRS space-time locations both with and without the AIRS quality control we estimate the sampling bias of the AIRS climatology and the atmospheric conditions where AIRS has a lower sampling rate. While the AIRS temperature and water vapor sampling biases are small at low latitudes, they can be more than a few degrees in temperature or 10 percent in water vapor at higher latitudes. The largest sampling biases are over desert. The AIRS and MERRA data are available from the Goddard Earth Sciences Data and Information Services Center (GES DISC). The AIRS climatologies we used are available for analysis with the GIOVANNI data exploration tool. (see, http://disc.gsfc.nasa.gov).

  6. Application of Satellite and Ground-based Data to Investigate the UV Radiative Effects of Australian Aerosols

    NASA Technical Reports Server (NTRS)

    Kalashnikova, Olga V.; Mills, Franklin P.; Eldering, Annmarie; Anderson, Don

    2007-01-01

    An understanding of the effect of aerosols on biologically- and photochemically-active UV radiation reaching the Earth's surface is important for many ongoing climate, biophysical, and air pollution studies. In particular, estimates of the UV characteristics of the most common Australian aerosols will be valuable inputs to UV Index forecasts, air quality studies, and assessments of the impact of regional environmental changes. By analyzing climatological distributions of Australian aerosols we have identified sites where co-located ground-based UV-B and ozone measurements were available during episodes of relatively high aerosol activity. Since at least June 2003, surface UV global irradiance spectra (285-450 nm) have been measured routinely at Darwin and Alice Springs in Australia by the Australian Bureau of Meteorology (BoM). Using colocated sunphotometer measurements at Darwin and Alice Springs, we identified several episodes of relatively high aerosol activity. Aerosol air mass types were analyzed from sunphotometer-derived angstrom parameter, MODIS fire maps and MISR aerosol property retrievals. To assess aerosol effects we compared the measured UV irradiances for aerosol-loaded and clear-sky conditions with each other and with irradiances simulated using the libRadtran radiative transfer model for aerosol-free conditions. We found that for otherwise similar atmospheric conditions, smoke aerosols over Darwin reduced the surface UV irradiance by as much as 40-50% at 290-300 nm and 20-25% at 320-400 nm near active fires (aerosol optical depth, AOD, at 500 nm approximately equal to 0.6). Downwind of fires, the smoke aerosols over Darwin reduced the surface irradiance by 15-25% at 290-300 nm and approximately 10% at 320-350 nm (AOD at 500 nm approximately equal to 0.2). The effect of smoke increased with decrease of wavel strongest in the UV-B. The aerosol attenuation factors calculated for the selected cases suggest smoke over Darwin has an effect on surface 340

  7. Climatic Effects of 1950-2050 Changes in US Anthropogenic Aerosols. Part 1; Aerosol Trends and Radiative Forcing

    NASA Technical Reports Server (NTRS)

    Leibensperger, E. M.; Mickley, L. J.; Jacob, D. J.; Chen, W.-T.; Seinfeld, J. H.; Nenes, A.; Adams, P. J.; Streets, D. G.; Kumar, N.; Rind, D.

    2012-01-01

    We calculate decadal aerosol direct and indirect (warm cloud) radiative forcings from US anthropogenic sources over the 1950-2050 period. Past and future aerosol distributions are constructed using GEOS-Chem and historical emission inventories and future projections from the IPCC A1B scenario. Aerosol simulations are evaluated with observed spatial distributions and 1980-2010 trends of aerosol concentrations and wet deposition in the contiguous US. Direct and indirect radiative forcing is calculated using the GISS general circulation model and monthly mean aerosol distributions from GEOS-Chem. The radiative forcing from US anthropogenic aerosols is strongly localized over the eastern US. We find that its magnitude peaked in 1970-1990, with values over the eastern US (east of 100 deg W) of -2.0Wm(exp-2 for direct forcing including contributions from sulfate (-2.0Wm-2), nitrate (-0.2Wm(exp-2), organic carbon (-0.2Wm(exp-2), and black carbon (+0.4Wm(exp-2). The uncertainties in radiative forcing due to aerosol radiative properties are estimated to be about 50 %. The aerosol indirect effect is estimated to be of comparable magnitude to the direct forcing. We find that the magnitude of the forcing declined sharply from 1990 to 2010 (by 0.8Wm(exp-2) direct and 1.0Wm(exp-2 indirect), mainly reflecting decreases in SO2 emissions, and project that it will continue declining post-2010 but at a much slower rate since US SO2 emissions have already declined by almost 60% from their peak. This suggests that much of the warming effect of reducing US anthropogenic aerosol sources has already been realized. The small positive radiative forcing from US BC emissions (+0.3Wm(exp-2 over the eastern US in 2010; 5% of the global forcing from anthropogenic BC emissions worldwide) suggests that a US emission control strategy focused on BC would have only limited climate benefit.

  8. Atmospheric Optical Properties and Spectral Analysis of Desert Aerosols

    NASA Astrophysics Data System (ADS)

    Yvgeni, D.; Karnieli, A.; Kaufman, Y. J.; Andreae, M. O.; Holben, B. N.; Maenhaut, W.

    2002-05-01

    Scientific background Aerosols can interact directly with solar and terrestrial radiation by scattering as well as absorption. In addition, they can indirectly alter the planetary albedo by modifying the properties of clouds. Objectives Investigations have been devoted to two main areas: (1) Aerosol climatology situation in the Negev desert, investigations of physical and chemical characteristics of aerosols, and study of the local and long-range transport trajectory of polluted air masses over the Negev desert; and (2) An estimation of the optical properties throughout the atmospheric column by surface measurements via performance of spectral and statistical analysis of the data received from two measurement systems. Results and conclusions Analyzed data from the Sede Boker site, in the Negev Desert of Israel, shows an increase in aerosol optical depth during the summer seasons and a decrease during winter. One of the possible reasons for this characteristic is an increase of the precipitable water (reaches 3.0-3.5 cm) due to a constant wind stream from the Mediterranean Sea in same time. The highest probability distribution of the aerosol optical depth is in the range of 0.15-0.20; and of the Angstrom parameter is in range of 0.83 - 1.07. During dust storm events, the scattering coefficient range at 670 nm and 440 nm wavelengths were inverted. It was discovered that the dust particles in this case had non-spherical character. Comparison between optical depth, measured through all atmospheric column, and scattering coefficient from surface measurements provides correlation coefficient (r) equal to 0.64. The Angstrom parameter, calculated via optical depth and via scattering coefficient, provides a correlation coefficient of 0.66. Thus we can obtain an estimate of the influence of the surface aerosol situation on column optical properties. The combined analysis of dust cloud altitude and optical depth as a function of the time indicates long-term transport and

  9. Aerosol Robotic Network (AERONET) Version 3 Aerosol Optical Depth and Inversion Products

    NASA Astrophysics Data System (ADS)

    Giles, D. M.; Holben, B. N.; Eck, T. F.; Smirnov, A.; Sinyuk, A.; Schafer, J.; Sorokin, M. G.; Slutsker, I.

    2017-12-01

    almucantar inversion database was computed using the NASA High End Computing resources at NASA Ames Research Center and NASA Goddard Space Flight Center. In addition to a description of data products, this presentation will provide a comparison of the V3 AOD and inversion climatology comparison of the V3 Level 2.0 and V2 Level 2.0 for sites with varying aerosol types.

  10. Climate forcing by anthropogenic aerosols

    NASA Technical Reports Server (NTRS)

    Charlson, R. J.; Schwartz, S. E.; Hales, J. M.; Cess, R. D.; Coakley, J. A., Jr.; Hansen, J. E.; Hofmann, D. J.

    1992-01-01

    Although long considered to be of marginal importance to global climate change, tropospheric aerosol contributes substantially to radiative forcing, and anthropogenic sulfate aerosol, in particular, has imposed a major perturbation to this forcing. Both the direct scattering of short-wavelength solar radiation and the modification of the shortwave reflective properties of clouds by sulfate aerosol particles increase planetary albedo, thereby exerting a cooling influence on the planet. Current climate forcing due to anthropogenic sulfate is estimated to be -1 to -2 watts per square meter, globally averaged. This perturbation is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign. Thus, the aerosol forcing has likely offset global greenhouse warming to a substantial degree. However, differences in geographical and seasonal distributions of these forcings preclude any simple compensation. Aerosol effects must be taken into account in evaluating anthropogenic influences on past, current, and projected future climate and in formulating policy regarding controls on emission of greenhouse gases and sulfur dioxide. Resolution of such policy issues requires integrated research on the magnitude and geographical distribution of aerosol climate forcing and on the controlling chemical and physical processes.

  11. Climate forcing by anthropogenic aerosols.

    PubMed

    Charlson, R J; Schwartz, S E; Hales, J M; Cess, R D; Coakley, J A; Hansen, J E; Hofmann, D J

    1992-01-24

    Although long considered to be of marginal importance to global climate change, tropospheric aerosol contributes substantially to radiative forcing, and anthropogenic sulfate aerosol in particular has imposed a major perturbation to this forcing. Both the direct scattering of shortwavelength solar radiation and the modification of the shortwave reflective properties of clouds by sulfate aerosol particles increase planetary albedo, thereby exerting a cooling influence on the planet. Current climate forcing due to anthropogenic sulfate is estimated to be -1 to -2 watts per square meter, globally averaged. This perturbation is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign. Thus, the aerosol forcing has likely offset global greenhouse warming to a substantial degree. However, differences in geographical and seasonal distributions of these forcings preclude any simple compensation. Aerosol effects must be taken into account in evaluating anthropogenic influences on past, current, and projected future climate and in formulating policy regarding controls on emission of greenhouse gases and sulfur dioxide. Resolution of such policy issues requires integrated research on the magnitude and geographical distribution of aerosol climate forcing and on the controlling chemical and physical processes.

  12. Extension and statistical analysis of the GACP aerosol optical thickness record

    NASA Astrophysics Data System (ADS)

    Geogdzhayev, Igor V.; Mishchenko, Michael I.; Li, Jing; Rossow, William B.; Liu, Li; Cairns, Brian

    2015-10-01

    The primary product of the Global Aerosol Climatology Project (GACP) is a continuous record of the aerosol optical thickness (AOT) over the oceans. It is based on channel-1 and -2 radiance data from the Advanced Very High Resolution Radiometer (AVHRR) instruments flown on successive National Oceanic and Atmospheric Administration (NOAA) platforms. We extend the previous GACP dataset by four years through the end of 2009 using NOAA-17 and -18 AVHRR radiances recalibrated against MODerate resolution Imaging Spectroradiometer (MODIS) radiance data, thereby making the GACP record almost three decades long. The temporal overlap of over three years of the new NOAA-17 and the previous NOAA-16 record reveals an excellent agreement of the corresponding global monthly mean AOT values, thereby confirming the robustness of the vicarious radiance calibration used in the original GACP product. The temporal overlap of the NOAA-17 and -18 instruments is used to introduce a small additive adjustment to the channel-2 calibration of the latter resulting in a consistent record with increased data density. The Principal Component Analysis (PCA) of the newly extended GACP record shows that most of the volcanic AOT variability can be isolated into one mode responsible for ~ 12% of the total variance. This conclusion is confirmed by a combined PCA analysis of the GACP, MODIS, and Multi-angle Imaging SpectroRadiometer (MISR) AOTs during the volcano-free period from February 2000 to December 2009. We show that the modes responsible for the tropospheric AOT variability in the three datasets agree well in terms of correlation and spatial patterns. A previously identified negative AOT trend which started in the late 1980s and continued into the early 2000s is confirmed. Its magnitude and duration indicate that it was caused by changes in tropospheric aerosols. The latest multi-satellite segment of the GACP record shows that this trend tapered off, with no noticeable AOT change after 2002. This

  13. Extension and Statistical Analysis of the GACP Aerosol Optical Thickness Record.

    NASA Technical Reports Server (NTRS)

    Geogdzhayev, Igor V.; Mishchenko, Michael I.; Li, Jing; Rossow, William B.; Liu, Li; Cairns, Brian

    2015-01-01

    The primary product of the Global Aerosol Climatology Project (GACP) is a continuous record of the aerosol optical thickness (AOT) over the oceans. It is based on channel-1 and -2 radiance data from the Advanced Very High Resolution Radiometer (AVHRR) instruments flown on successive National Oceanic and Atmospheric Administration (NOAA) platforms. We extend the previous GACP dataset by four years through the end of 2009 using NOAA-17 and -18 AVHRR radiances recalibrated against MODerate resolution Imaging Spectroradiometer (MODIS) radiance data, thereby making the GACP record almost three decades long. The temporal overlap of over three years of the new NOAA-17 and the previous NOAA-16 record reveals an excellent agreement of the corresponding global monthly mean AOT values, thereby confirming the robustness of the vicarious radiance calibration used in the original GACP product. The temporal overlap of the NOAA-17 and -18 instruments is used to introduce a small additive adjustment to the channel-2 calibration of the latter resulting in a consistent record with increased data density. The Principal Component Analysis (PCA) of the newly extended GACP record shows that most of the volcanic AOT variability can be isolated into one mode responsible for 12% of the total variance. This conclusion is confirmed by a combined PCA analysis of the GACP, MODIS, andMulti-angle Imaging SpectroRadiometer (MISR) AOTs during the volcano-free period fromFebruary 2000 to December 2009.We show that the modes responsible for the tropospheric AOT variability in the three datasets agree well in terms of correlation and spatial patterns. A previously identified negative AOT trend which started in the late 1980s and continued into the early 2000s is confirmed. Its magnitude and duration indicate that it was caused by changes in tropospheric aerosols. The latest multi-satellite segment of the GACP record shows that this trend tapered off, with no noticeable AOT change after 2002. This

  14. Multi-Sensory Aerosol Data and the NRL NAAPS model for Regulatory Exceptional Event Analysis

    NASA Astrophysics Data System (ADS)

    Husar, R. B.; Hoijarvi, K.; Westphal, D. L.; Haynes, J.; Omar, A. H.; Frank, N. H.

    2013-12-01

    Beyond scientific exploration and analysis, multi-sensory observations along with models are finding increasing applications for operational air quality management. EPA's Exceptional Event (EE) Rule allows the exclusion of data strongly influenced by impacts from "exceptional events," such as smoke from wildfires or dust from abnormally high winds. The EE Rule encourages the use of satellite observations and other non-standard data along with models as evidence for formal documentation of EE samples for exclusion. Thus, the implementation of the EE Rule is uniquely suited for the direct application of integrated multi-sensory observations and indirectly through the assimilation into an aerosol simulation model. Here we report the results of a project: NASA and NAAPS Products for Air Quality Decision Making. The project uses of observations from multiple satellite sensors, surface-based aerosol measurements and the NRL Aerosol Analysis and Prediction System (NAAPS) model that assimilates key satellite observations. The satellite sensor data for detecting and documenting smoke and dust events include: MODIS AOD and Images; OMI Aerosol Index, Tropospheric NO2; AIRS, CO. The surface observations include the EPA regulatory PM2.5 network; the IMPROVE/STN aerosol chemical network; AIRNOW PM2.5 mass network, and surface met. data. Within this application, crucial role is assigned to the NAAPS model for estimating the surface concentration of windblown dust and biomass smoke. The operational model assimilates quality-assured daily MODIS data and 2DVAR to adjust the model concentrations and CALIOP-based climatology to adjust the vertical profiles at 6-hour intervals. The assimilation of satellite data from multiple satellites significantly contributes to the usefulness of NAAPS for EE analysis. The NAAPS smoke and dust simulations were evaluated using the IMPROVE/STN chemical data. The multi-sensory observations along with the model simulations are integrated into a web

  15. Relating the dynamics of climatological and hydrological droughts in semiarid Botswana

    NASA Astrophysics Data System (ADS)

    Byakatonda, Jimmy; Parida, B. P.; Kenabatho, Piet K.

    2018-06-01

    Dynamics of droughts have been an associated feature of climate variability particularly in semiarid regions which impact on the response of hydrological systems. This study attempts to determine drought timescale that is suitable for monitoring the effects of drought on hydrological systems which can then be used to assess the long term persistence or reversion and forecasts of the dynamics. Based on this, climatological and hydrological drought indices characterized by Standardized precipitation evapotranspiration index (SPEI) and Standardized flow index (SFI) respectively have been determined using monthly rainfall, temperature and flow data from two major river systems. The association between climatological and hydrological droughts in Botswana has been investigated using these river systems namely: Okavango that is predominantly a storage type and Limpopo which is non-storage for a period of 1975-2014. Dynamics of climatological and hydrological droughts are showing trends towards drying conditions at both river systems. It was also observed that hydrological droughts lag climatological droughts by 7 months in Limpopo and 6 months in Okavango river systems respectively. Analyses of the association between climatic and flow indices indicate that the degree of association becomes stronger with increasing timescale at the Okavango river system. However in the Limpopo river system, it was observed that high timescales of 18- and 24-months were not useful in drought monitoring. 15-months timescale was identified to best monitor drought dynamics at both locations. Therefore SPEIs and SFIs computed at 15-months timescale have been used to assess the variability and long term persistence in drought dynamics through rescaled range analysis (R/S). H-coefficients of 0.06 and 0.08 resulted for Limpopo and Okavango respectively. These H-coefficients being significantly less than 0.5 is an indication of high variability and suggests a change in dynamics from the existing

  16. Modeling the Influences of Aerosols on Pre-Monsoon Circulation and Rainfall over Southeast Asia

    NASA Technical Reports Server (NTRS)

    Lee, D.; Sud, Y. C.; Oreopoulos, L.; Kim, K.-M.; Lau, W. K.; Kang, I.-S.

    2014-01-01

    We conduct several sets of simulations with a version of NASA's Goddard Earth Observing System, version 5, (GEOS-5) Atmospheric Global Climate Model (AGCM) equipped with a two-moment cloud microphysical scheme to understand the role of biomass burning aerosol (BBA) emissions in Southeast Asia (SEA) in the pre-monsoon period of February-May. Our experiments are designed so that both direct and indirect aerosol effects can be evaluated. For climatologically prescribed monthly sea surface temperatures, we conduct sets of model integrations with and without biomass burning emissions in the area of peak burning activity, and with direct aerosol radiative effects either active or inactive. Taking appropriate differences between AGCM experiment sets, we find that BBA affects liquid clouds in statistically significantly ways, increasing cloud droplet number concentrations, decreasing droplet effective radii (i.e., a classic aerosol indirect effect), and locally suppressing precipitation due to a deceleration of the autoconversion process, with the latter effect apparently also leading to cloud condensate increases. Geographical re-arrangements of precipitation patterns, with precipitation increases downwind of aerosol sources are also seen, most likely because of advection of weakly precipitating cloud fields. Somewhat unexpectedly, the change in cloud radiative effect (cloud forcing) at surface is in the direction of lesser cooling because of decreases in cloud fraction. Overall, however, because of direct radiative effect contributions, aerosols exert a net negative forcing at both the top of the atmosphere and, perhaps most importantly, the surface, where decreased evaporation triggers feedbacks that further reduce precipitation. Invoking the approximation that direct and indirect aerosol effects are additive, we estimate that the overall precipitation reduction is about 40% due to the direct effects of absorbing aerosols, which stabilize the atmosphere and reduce

  17. A study of aerosol indirect effects and feedbacks on convective precipitation

    NASA Astrophysics Data System (ADS)

    Da Silva, Nicolas; Mailler, Sylvain; Drobinski, Philippe

    2017-04-01

    Atmospheric aerosols from natural and anthropogenic origin are present in the troposphere of the Mediterranean basin and continental Europe, occasionnally reaching very high concentrations in air masses with a strong content of aerosols related to mineral dust emissions, wildfires, or anthropogenic contamination [1]. On the other hand precipitations in the Mediterranean basin need to be understood precisely since drought and extreme precipitation events are a part of Mediterranean climate which can strongly affect the people and the economic activity in the Mediterranean basin [2]. The present study is a contribution to the investigations on the effects of aerosols on precipitation in the Mediterranean basin and continental Europe. For that purpose, we used the Weather Research and Forecasting Model (WRF) parameterized with the Thompson aerosol-aware microphysics schemes, performing two sensitivity simulations forced with two different aerosol climatologies during six months covering an entire summer season on a domain, covering the Mediterranean basin and continental Europe at 50 km resolution. Aerosols may affect atmospheric dynamics through their direct and semidirect radiative effects as well as through their indirect effects (through the changes of cloud microphysics). While it is difficult to disentangle these differents effects in reality, numerical modelling with the WRF model make it possible to isolate indirect effects by modifying them without affecting the direct or semidirect effects of aerosols in an attempt to examine the effect of aerosols on precipitations through microphysical effects only. Our first results have shown two opposite responses depending whether the precipitation are convective or large-scale. Since convective precipitations seem to be clearly inhibited by increased concentrations of cloud-condensation nuclei, we attempted to understand which processes and feedbacks are involved in this reduction of parameterized convective

  18. Aerosols in coastal and inland areas in the equatorial African belt.

    PubMed

    Ssenyonga, Taddeo; Muyimbwa, Dennis; Okullo, Willy; Chen, Yi-Chun; Frette, Øvyind; Hamre, Børge; Steigen, Andreas; Dahlback, Arne; Stamnes, Jakob J

    2014-05-10

    Aerosols affect the climate directly through absorption and reflection of sunlight back to space and indirectly by acting as cloud condensation nuclei. This paper is based on more than three decades of satellite data (1979-1994 and 1996-2012) from total ozone mapping spectrometer (TOMS) and ozone monitoring instrument (OMI), which have provided measurements of backscattered radiances in the wavelength range from 331 to 380 nm. These data have been used to determine the aerosol climatology and to investigate the influence of the aerosol index (AI) on the ultraviolet index (UVI) in coastal land areas in Serrekunda (13.28°N, 16.34°W), The Gambia, and Dar-es-Salaam (6.8°S, 39.26°E), Tanzania, as well as in inland areas in Kampala (0.19°N, 32.34°E), Uganda. Heavy aerosol loadings were found to occur in the dry seasons at all three locations. To reduce the influence of clouds, we disregarded TOMS and OMI data for days during which the UV reflectivity was larger than 9% and investigated the correlation of the AI with the UVI for the remaining days at the three locations. We found a high correlation coefficient of 0.82 for Serrekunda, but poor correlation for Kampala and Dar-es-Salaam. The average AI for Serrekunda was found to be about three times higher than that for Kampala or Dar-es-Salaam, and a positive trend was found for the AI in Kampala and Dar-es-Salaam, whereas a negative trend was found for the AI in Serrekunda.

  19. Aerosol particle size distribution in the stratosphere retrieved from SCIAMACHY limb measurements

    NASA Astrophysics Data System (ADS)

    Malinina, Elizaveta; Rozanov, Alexei; Rozanov, Vladimir; Liebing, Patricia; Bovensmann, Heinrich; Burrows, John P.

    2018-04-01

    aerosols in the Earth's atmosphere is of a great importance in the scientific community. While tropospheric aerosol influences the radiative balance of the troposphere and affects human health, stratospheric aerosol plays an important role in atmospheric chemistry and climate change. In particular, information about the amount and distribution of stratospheric aerosols is required to initialize climate models, as well as validate aerosol microphysics models and investigate geoengineering. In addition, good knowledge of stratospheric aerosol loading is needed to increase the retrieval accuracy of key trace gases (e.g. ozone or water vapour) when interpreting remote sensing measurements of the scattered solar light. The most commonly used characteristics to describe stratospheric aerosols are the aerosol extinction coefficient and Ångström coefficient. However, the use of particle size distribution parameters along with the aerosol number density is a more optimal approach. In this paper we present a new retrieval algorithm to obtain the particle size distribution of stratospheric aerosol from space-borne observations of the scattered solar light in the limb-viewing geometry. While the mode radius and width of the aerosol particle size distribution are retrieved, the aerosol particle number density profile remains unchanged. The latter is justified by a lower sensitivity of the limb-scattering measurements to changes in this parameter. To our knowledge this is the first data set providing two parameters of the particle size distribution of stratospheric aerosol from space-borne measurements of scattered solar light. Typically, the mode radius and w can be retrieved with an uncertainty of less than 20 %. The algorithm was successfully applied to the tropical region (20° N-20° S) for 10 years (2002-2012) of SCIAMACHY observations in limb-viewing geometry, establishing a unique data set. Analysis of this new climatology for the particle size

  20. Simultaneously inferring above-cloud absorbing aerosol optical thickness and underlying liquid phase cloud optical and microphysical properties using MODIS

    NASA Astrophysics Data System (ADS)

    Meyer, Kerry; Platnick, Steven; Zhang, Zhibo

    2015-06-01

    The regional haze over the southeast (SE) Atlantic Ocean induced by biomass burning in southern Africa can be problematic for passive imager-based retrievals of the underlying quasi-permanent marine boundary layer (MBL) clouds and for estimates of top-of-atmosphere (TOA) aerosol direct radiative effect (DRE). Here an algorithm is introduced to simultaneously retrieve above-cloud aerosol optical thickness (AOT), the cloud optical thickness (COT), and cloud effective particle radius (CER) of the underlying MBL clouds while also providing pixel-level estimates of retrieval uncertainty. This approach utilizes reflectance measurements at six Moderate Resolution Imaging Spectroradiometer (MODIS) channels from the visible to the shortwave infrared. Retrievals are run under two aerosol model assumptions on 8 years (2006-2013) of June-October Aqua MODIS data over the SE Atlantic, from which a regional cloud and above-cloud aerosol climatology is produced. The cloud retrieval methodology is shown to yield COT and CER consistent with those from the MODIS operational cloud product (MOD06) when forcing AOT to zero, while the full COT-CER-AOT retrievals that account for the above-cloud aerosol attenuation increase regional monthly mean COT and CER by up to 9% and 2%, respectively. Retrieved AOT is roughly 3 to 5 times larger than the collocated 532 nm Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) retrievals, though closer agreement is observed with the CALIOP 1064 nm retrievals, a result consistent with previous case study analyses. Regional cloudy-sky above-cloud aerosol DRE calculations are also performed that illustrate the importance of the aerosol model assumption and underlying cloud retrievals.

  1. Aerosol radiative effects and their trends under clear-sky situations over Europe

    NASA Astrophysics Data System (ADS)

    Bartok, Blanka

    2017-04-01

    In the literature great uncertainties ca be found regarding radiative effects of aerosols on the energy budget of the atmosphere (IPCC, 2013). In the study the aerosols radiative effects on clear-sky solar radiation are quantified over Europe using empirical and physical modelling approaches. The values of aerosol radiation effect are determined by the MAGIC radiation code. In the first run clear-sky radiation is calculated integrating KINEE/MPI/Aerocom aerosol climatology and ERA-INTERIM water vapour multiannual monthly means. In the next run the clear-sky radiation are also calculated ignoring aerosol data (adjusted to 0) from the algorithm. Both runs were carried out for each months of the year, taking into account the varying astrological factors. The difference between the aerosol-included and aerosol-free clear-sky radiation is equal to the absolute aerosol radiative effect in W/m2. The annual mean of the surface aerosol radiative effects in clear-sky situations over Europe is -7.1 ± 2.9 W/m2, high values are representing the central part of the continent and the Mediterranean Basin. Furthermore the trends of the aerosol radiative effects are also determined for the period of 2001-2012. First a linear fitting is elaborated between the aerosol optical depth (AOT) built in the MAGIC code and its aerosol radiative effect calculated by the code. Next, based on these linear functions a radiative effect values are assigned to each monthly AOT500 value available from the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra Level-3 experiment. In this way a new dataset of aerosol radiative effect for the period of 2001-2012 has been created. Beside of this approach the changes in aerosol radiative effects are also calculated based on ground-based clear-sky radiation trends. This approach is used as a validation of the method applied in earlier stage, mainly for the linear fitting. The starting point of this approach is to elaborate the trends of clear

  2. Intercomparison of aerosol-cloud-precipitation interactions in stratiform orographic mixed-phase clouds

    NASA Astrophysics Data System (ADS)

    Muhlbauer, A.; Hashino, T.; Xue, L.; Teller, A.; Lohmann, U.; Rasmussen, R. M.; Geresdi, I.; Pan, Z.

    2010-09-01

    . Furthermore, it is found that neither a decrease in cloud droplet coalescence nor a decrease in riming necessarily implies a decrease in precipitation due to compensation effects by other microphysical pathways. The simulations suggest that mixed-phase conditions play an important role in buffering the effect of aerosol perturbations on cloud microphysics and reducing the overall susceptibility of clouds and precipitation to changes in the aerosol number concentrations. As a consequence the aerosol effect on precipitation is suggested to be less pronounced or even inverted in regions with high terrain (e.g., the Alps or Rocky Mountains) or in regions where mixed-phase microphysics is important for the climatology of orographic precipitation.

  3. Disentangling sea-surface temperature and anthropogenic aerosol influences on recent trends in South Asian monsoon rainfall

    NASA Astrophysics Data System (ADS)

    Patil, Nitin; Venkataraman, Chandra; Muduchuru, Kaushik; Ghosh, Subimal; Mondal, Arpita

    2018-05-01

    Recent studies point to combined effects of changes in regional land-use, anthropogenic aerosol forcing and sea surface temperature (SST) gradient on declining trends in the South Asian monsoon (SAM). This study attempted disentangling the effects produced by changes in SST gradient from those by aerosol levels in an atmospheric general circulation model. Two pairs of transient ensemble simulations were made, for a 40-year period from 1971 to 2010, with evolving versus climatological SSTs and with anthropogenic aerosol emissions fixed at 1971 versus 2010, in each case with evolution of the other forcing element, as well as GHGs. Evolving SST was linked to a widespread feedback on increased surface temperature, reduced land-sea thermal contrast and a weakened Hadley circulation, with weakening of cross-equatorial transport of moisture transport towards South Asia. Increases in anthropogenic aerosol levels (1971 versus 2010), led to an intensification of drying in the peninsular Indian region, through several regional pathways. Aerosol forcing induced north-south asymmetries in temperature and sea-level pressure response, and a cyclonic circulation in the Bay of Bengal, leading to an easterly flow, which opposes the monsoon flow, suppressing moisture transport over peninsular India. Further, aerosol induced decreases in convection, vertically integrated moisture flux convergence, evaporation flux and cloud fraction, in the peninsular region, were spatially congruent with reduced convective and stratiform rainfall. Overall, evolution of SST acted through a weakening of cross-equatorial moisture flow, while increases in aerosol levels acted through suppression of Arabian Sea moisture transport, as well as, of convection and vertical moisture transport, to influence the suppression of SAM rainfall.

  4. Transport and recirculation of aerosols off Southern Africa—macroscale plume structure

    NASA Astrophysics Data System (ADS)

    Tyson, P. D.; D'Abreton, P. C.

    A pall of aerosols and trace gases frequently occurs over southern Africa to a depth of ˜500 hPa, blanketing vast areas, particularly in the austral winter and spring. Large-scale offshore transport of these aerosols and trace gases in extremely large plumes from interior continental areas of the subcontinent to the Indian and Atlantic Oceans is a common occurrence. The nature of the transport plumes, their climatology, chemical composition and morphology are discussed. In the vertically integrated, surface-to-500 hPa layer, poleward of about 15° S, transport into the Indian Ocean is shown to be about 60% greater into the Indian Ocean than into the Atlantic Ocean. Recirculation of atmospheric constituents is considered and estimates of aerosol mass fluxes over central southern Africa are presented. Of the total of about 50 Mt yr -1 of aerosols being transported at the central meridian, 44% is shown to be recirculated material. The rest exits the subcontinent directly without recirculation. Preferred plume corridors of exit and entry are postulated for different localities on the east and west coasts. Two case studies of east- and west-coast plumes apparently flowing uniformly out of southern Africa are examined. The illusion of uniformity in plume structure is shown to be misleading. Both plumes are shown to be above and separated from the marine boundary layer. Each is over 1500 km in width and 3-5 km deep. Likewise, both are capped by absolutely stable layers at ˜500 hPa and exhibit a complex structure of both outflowing aerosols and trace gases and inflowing, recycled and recirculated material. Indications of the composition of the recirculated material are given and implications of the plume transports are considered.

  5. Pretest aerosol code comparisons for LWR aerosol containment tests LA1 and LA2

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wright, A.L.; Wilson, J.H.; Arwood, P.C.

    The Light-Water-Reactor (LWR) Aerosol Containment Experiments (LACE) are being performed in Richland, Washington, at the Hanford Engineering Development Laboratory (HEDL) under the leadership of an international project board and the Electric Power Research Institute. These tests have two objectives: (1) to investigate, at large scale, the inherent aerosol retention behavior in LWR containments under simulated severe accident conditions, and (2) to provide an experimental data base for validating aerosol behavior and thermal-hydraulic computer codes. Aerosol computer-code comparison activities are being coordinated at the Oak Ridge National Laboratory. For each of the six LACE tests, ''pretest'' calculations (for code-to-code comparisons) andmore » ''posttest'' calculations (for code-to-test data comparisons) are being performed. The overall goals of the comparison effort are (1) to provide code users with experience in applying their codes to LWR accident-sequence conditions and (2) to evaluate and improve the code models.« less

  6. Daytime variation of aerosol optical depth in North China and its impact on aerosol direct radiative effects

    NASA Astrophysics Data System (ADS)

    Song, Jingjing; Xia, Xiangao; Che, Huizheng; Wang, Jun; Zhang, Xiaoling; Li, Xiaojing

    2018-06-01

    Daytime cycles of aerosol optical depth (AOD) and Angstrom exponent (AE) climatology were analyzed based on long-term (5-15 years) measurements at 18 stations of the China Aerosol Remote Sensing Network (CARSNET) in North China. AOD in Northwest China (NWC) exhibits a daytime trend with negative departures in the early morning and later afternoon while positive departures at midday. Daytime AOD relative departure in different sites and seasons varies from -30.26% to 30.28%. AE in NWC shows an opposite pattern to daytime variation of AOD. Daytime variation of AE is negligible in North China Plain (NCP), AOD increases steadily throughout the day. This trend is consistent and repeatable in four seasons. Such pronounced variability in AOD and AE should be taken accounted for in the estimation of diurnal aerosol direct radiative effects (ADRE), as suggested by the radiative transfer model simulations. The replacement of the observed daytime variation of AOD and AE by daytime mean values in NWC results in ADRE differences of 0.31 Wm-2 at the surface and 0.05 Wm-2 at the top of the atmosphere (TOA). ADRE in NWC will be underestimated by -0.47 Wm-2 and -0.25 Wm-2 at the surface and TOA, respectively, if instantaneous AOD and AE during the overpass time of Terra and Aqua are taken as the daytime mean values. The annual mean ADRE at the surface and TOA will be underestimated by -0.17 Wm-2 and -0.03 Wm-2 if daytime variations of AOD and AE are replaced by daytime mean values in NCP. ADRE will be underestimated by -0.07 Wm-2 at the surface and -0.06 Wm-2 at the TOA if instantaneous AOD and AE during the overpass time of Terra and Aqua other than daytime variation of AOD and AE are used in the calculations.

  7. Comparative climatology of four marine stratocumulus regimes

    NASA Technical Reports Server (NTRS)

    Hanson, Howard P.

    1990-01-01

    The climatology of marine stratocumulus (MSc) cloud regimes off the west coasts of California, Peru, Morocco, and Angola are examined. Long-term, annual averages are presented for several quantities of interest in the four MSc regimes. The climatologies were constructed using the Comprehensive Ocean-Atmosphere Data Set (COADS). A 40 year time series of observations was extracted for 32 x 32 deg analysis domains. The data were taken from the monthly-averaged, 2 deg product. The resolution of the analysis is therefore limited to scales of greater than 200 km with submonthly variability not resolved. The averages of total cloud cover, sea surface temperature, and surface pressure are presented.

  8. Satellite Ocean Aerosol Retrieval (SOAR) Algorithm Extension to S-NPP VIIRS as Part of the "Deep Blue" Aerosol Project

    NASA Astrophysics Data System (ADS)

    Sayer, A. M.; Hsu, N. C.; Lee, J.; Bettenhausen, C.; Kim, W. V.; Smirnov, A.

    2018-01-01

    The Suomi National Polar-Orbiting Partnership (S-NPP) satellite, launched in late 2011, carries the Visible Infrared Imaging Radiometer Suite (VIIRS) and several other instruments. VIIRS has similar characteristics to prior satellite sensors used for aerosol optical depth (AOD) retrieval, allowing the continuation of space-based aerosol data records. The Deep Blue algorithm has previously been applied to retrieve AOD from Sea-viewing Wide Field-of-view Sensor (SeaWiFS) and Moderate Resolution Imaging Spectroradiometer (MODIS) measurements over land. The SeaWiFS Deep Blue data set also included a SeaWiFS Ocean Aerosol Retrieval (SOAR) algorithm to cover water surfaces. As part of NASA's VIIRS data processing, Deep Blue is being applied to VIIRS data over land, and SOAR has been adapted from SeaWiFS to VIIRS for use over water surfaces. This study describes SOAR as applied in version 1 of NASA's S-NPP VIIRS Deep Blue data product suite. Several advances have been made since the SeaWiFS application, as well as changes to make use of the broader spectral range of VIIRS. A preliminary validation against Maritime Aerosol Network (MAN) measurements suggests a typical uncertainty on retrieved 550 nm AOD of order ±(0.03+10%), comparable to existing SeaWiFS/MODIS aerosol data products. Retrieved Ångström exponent and fine-mode AOD fraction are also well correlated with MAN data, with small biases and uncertainty similar to or better than SeaWiFS/MODIS products.

  9. The DACCIWA Project: Dynamics-Aerosol-Chemistry-Cloud interactions in West Africa

    NASA Astrophysics Data System (ADS)

    Knippertz, Peter

    2014-05-01

    Massive economic and population growth and urbanisation are expected to lead to a tripling of anthropogenic emissions from southern West Africa (SWA) between 2000 and 2030, the impacts of which on human health, ecosystems, food security and the regional climate are largely unknown. An assessment of these impacts is complicated by (a) a superposition with effects of global climate change, (b) the strong dependence of SWA on the sensitive West African monsoon, (c) incomplete scientific understanding of interactions between emissions, clouds, radiation, precipitation and regional circulations and (d) by a lack of observations to advance our understanding and improve predictions. The purpose of this contribution is to introduce the research consortium DACCIWA (Dynamics-Aerosol-Chemistry-Cloud interactions in West Africa), which comprises 16 partners in six European and West African countries. The interdisciplinary DACCIWA team will build on the scientific and logistical foundations established by the African Monsoon Multidisciplinary Analysis (AMMA) project and collaborate closely with operational centres. DACCIWA will receive funding of about M8.75€ from the European Commission as part of Framework Programme 7 from 2015 until 2018. The DACCIWA project will conduct extensive fieldwork in SWA to collect high-quality observations, spanning the entire process chain from surface-based natural and anthropogenic emissions to impacts on health, ecosystems and climate. This will include a major field campaign in summer 2015 with three research aircrafts and two ground-based supersites. Combining the resulting benchmark dataset with a wide range of modelling activities will allow us: (a) to assess all relevant physical and chemical processes, (b) to improve the monitoring of climate and compositional parameters from space, (c) to determine health impacts from air pollution, and (d) to develop the next generation of weather and climate models capable of representing coupled

  10. Aerosol Optical Depths over Oceans: a View from MISR Retrievals and Collocated MAN and AERONET in Situ Observations

    NASA Technical Reports Server (NTRS)

    Witek, Marcin L.; Garay, Michael J.; Diner, David J.; Smirnov, Alexander

    2013-01-01

    In this study, aerosol optical depths over oceans are analyzed from satellite and surface perspectives. Multiangle Imaging SpectroRadiometer (MISR) aerosol retrievals are investigated and validated primarily against Maritime Aerosol Network (MAN) observations. Furthermore, AErosol RObotic NETwork (AERONET) data from 19 island and coastal sites is incorporated in this study. The 270 MISRMAN comparison points scattered across all oceans were identified. MISR on average overestimates aerosol optical depths (AODs) by 0.04 as compared to MAN; the correlation coefficient and root-mean-square error are 0.95 and 0.06, respectively. A new screening procedure based on retrieval region characterization is proposed, which is capable of substantially reducing MISR retrieval biases. Over 1000 additional MISRAERONET comparison points are added to the analysis to confirm the validity of the method. The bias reduction is effective within all AOD ranges. Setting a clear flag fraction threshold to 0.6 reduces the bias to below 0.02, which is close to a typical ground-based measurement uncertainty. Twelve years of MISR data are analyzed with the new screening procedure. The average over ocean AOD is reduced by 0.03, from 0.15 to 0.12. The largest AOD decrease is observed in high latitudes of both hemispheres, regions with climatologically high cloud cover. It is postulated that the screening procedure eliminates spurious retrieval errors associated with cloud contamination and cloud adjacency effects. The proposed filtering method can be used for validating aerosol and chemical transport models.

  11. Lidar Observations of Tropospheric Aerosols Over Northeastern South Africa During the ARREX and SAFARI-2000 Dry Season Experiments

    NASA Technical Reports Server (NTRS)

    Campbell, James R.; Welton, Ellsworth J.; Spinhirne, James D.; Ji, Qiang; Tsay, Si-Chee; Piketh, Stuart J.; Barenbrug, Marguerite; Holben, Brent; Starr, David OC. (Technical Monitor)

    2002-01-01

    During the ARREX-1999 and SAFARI-2000 Dry Season experiments a micropulse lidar (523 nm) instrument was operated at the Skukuza Airport in northeastern South Africa. The Mar was collocated with a diverse array of passive radiometric equipment. For SAFARI-2000 the processed Mar data yields a daytime time-series of layer mean/derived aerosol optical properties, including extinction-to-backscatter ratios and vertical extinction cross-section profile. Combined with 523 run aerosol optical depth and spectral Angstrom exponent calculations from available CIMEL sun-photometer data and normalized broadband flux measurements the temporal evolution of the near surface aerosol layer optical properties is analyzed for climatological trends. For the densest smoke/haze events the extinction-to-backscatter ratio is found to be between 60-80/sr, and corresponding Angstrom exponent calculations near and above 1.75. The optical characteristics of an evolving smoke event from SAFARI-2000 are extensively detailed. The advecting smoke was embedded within two distinct stratified thermodynamic layers, causing the particulate mass to advect over the instrument array in an incoherent manner on the afternoon of its occurrence. Surface broadband flux forcing due to the smoke is calculated, as is the evolution in the vertical aerosol extinction profile as measured by the Han Finally, observations of persistent elevated aerosol during ARREX-1999 are presented and discussed. The lack of corroborating observations the following year makes these observation; both unique and noteworthy in the scope of regional aerosol transport over southern Africa.

  12. Situational Lightning Climatologies for Central Florida: Phase IV: Central Florida Flow Regime Based Climatologies of Lightning Probabilities

    NASA Technical Reports Server (NTRS)

    Bauman, William H., III

    2009-01-01

    The threat of lightning is a daily concern during the warm season in Florida. Research has revealed distinct spatial and temporal distributions of lightning occurrence that are strongly influenced by large-scale atmospheric flow regimes. Previously, the Applied Meteorology Unit (AMU) calculated the gridded lightning climatologies based on seven flow regimes over Florida for 1-, 3- and 6-hr intervals in 5-, 10-, 20-, and 30-NM diameter range rings around the Shuttle Landing Facility (SLF) and eight other airfields in the National Weather Service in Melbourne (NWS MLB) county warning area (CWA). In this update to the work, the AMU recalculated the lightning climatologies for using individual lightning strike data to improve the accuracy of the climatologies. The AMU included all data regardless of flow regime as one of the stratifications, added monthly stratifications, added three years of data to the period of record and used modified flow regimes based work from the AMU's Objective Lightning Probability Forecast Tool, Phase II. The AMU made changes so the 5- and 10-NM radius range rings are consistent with the aviation forecast requirements at NWS MLB, while the 20- and 30-NM radius range rings at the SLF assist the Spaceflight Meteorology Group in making forecasts for weather Flight Rule violations during Shuttle landings. The AMU also updated the graphical user interface with the new data.

  13. Climatologies at high resolution for the earth's land surface areas

    NASA Astrophysics Data System (ADS)

    Karger, Dirk Nikolaus; Conrad, Olaf; Böhner, Jürgen; Kawohl, Tobias; Kreft, Holger; Soria-Auza, Rodrigo Wilber; Zimmermann, Niklaus E.; Linder, H. Peter; Kessler, Michael

    2017-09-01

    High-resolution information on climatic conditions is essential to many applications in environmental and ecological sciences. Here we present the CHELSA (Climatologies at high resolution for the earth's land surface areas) data of downscaled model output temperature and precipitation estimates of the ERA-Interim climatic reanalysis to a high resolution of 30 arc sec. The temperature algorithm is based on statistical downscaling of atmospheric temperatures. The precipitation algorithm incorporates orographic predictors including wind fields, valley exposition, and boundary layer height, with a subsequent bias correction. The resulting data consist of a monthly temperature and precipitation climatology for the years 1979-2013. We compare the data derived from the CHELSA algorithm with other standard gridded products and station data from the Global Historical Climate Network. We compare the performance of the new climatologies in species distribution modelling and show that we can increase the accuracy of species range predictions. We further show that CHELSA climatological data has a similar accuracy as other products for temperature, but that its predictions of precipitation patterns are better.

  14. Aerosol Modeling for the Global Model Initiative

    NASA Technical Reports Server (NTRS)

    Weisenstein, Debra K.; Ko, Malcolm K. W.

    2001-01-01

    The goal of this project is to develop an aerosol module to be used within the framework of the Global Modeling Initiative (GMI). The model development work will be preformed jointly by the University of Michigan and AER, using existing aerosol models at the two institutions as starting points. The GMI aerosol model will be tested, evaluated against observations, and then applied to assessment of the effects of aircraft sulfur emissions as needed by the NASA Subsonic Assessment in 2001. The work includes the following tasks: 1. Implementation of the sulfur cycle within GMI, including sources, sinks, and aqueous conversion of sulfur. Aerosol modules will be added as they are developed and the GMI schedule permits. 2. Addition of aerosol types other than sulfate particles, including dust, soot, organic carbon, and black carbon. 3. Development of new and more efficient parameterizations for treating sulfate aerosol nucleation, condensation, and coagulation among different particle sizes and types.

  15. Investigation of shortcomings in simulated aerosol vertical profiles

    NASA Astrophysics Data System (ADS)

    Park, S.; Allen, R.

    2017-12-01

    The vertical distribution of aerosols is one important factor for aerosol radiative forcing. Previous studies show that climate models poorly reproduce the aerosol vertical profile, with too much aerosol aloft in the upper troposphere. This bias may be related to several factors, including excessive convective mass flux and wet removal. In this study, we evaluate the aerosol vertical profile from several Coupled Model Intercomparison Project 5 (CMIP5) models, as well as the Community Atmosphere Model 5 (CAM5), relative to the Cloud-Aerosol Lidar Infrared Pathfinder Satellite Observation (CALIPSO). The results show that all models significantly underestimate extinction coefficient in the lower troposphere, while overestimating extinction coefficient in the upper troposphere. In addition, the majority of models indicate a land-ocean dependence in the relationship between aerosol extinction coefficient in the upper troposphere and convective mass flux. Over the continents, more convective mass flux is related to more aerosol aloft; over the ocean, more convective mass flux is associated with less aerosol in upper troposphere. Sensitivity experiments are conducted to investigate the role that convection and wet deposition have in contributing to the deficient simulation of the vertical aerosol profile, including the land-ocean dependence.

  16. Assessing a Tornado Climatology from Global Tornado Intensity Distributions.

    NASA Astrophysics Data System (ADS)

    Feuerstein, Bernold; Dotzek, Nikolai; Grieser, Jürgen

    2005-02-01

    Recent work demonstrated that the shape of tornado intensity distributions from various regions worldwide is well described by Weibull functions. This statistical modeling revealed a strong correlation between the fit parameters c for shape and b for scale regardless of the data source. In the present work it is shown that the quality of the Weibull fits is optimized if only tornado reports of F1 and higher intensity are used and that the c-b correlation does indeed reflect a universal feature of the observed tornado intensity distributions. For regions with likely supercell tornado dominance, this feature is the number ratio of F4 to F3 tornado reports R(F4/F3) = 0.238. The c-b diagram for the Weibull shape and scale parameters is used as a climatological chart, which allows different types of tornado climatology to be distinguished, presumably arising from supercell versus nonsupercell tornadogenesis. Assuming temporal invariance of the climatology and using a detection efficiency function for tornado observations, a stationary climatological probability distribution from large tornado records (U.S. decadal data 1950-99) is extracted. This can be used for risk assessment, comparative studies on tornado intensity distributions worldwide, and estimates of the degree of underreporting for areas with poor databases. For the 1990s U.S. data, a likely tornado underreporting of the weak events (F0, F1) by a factor of 2 can be diagnosed, as well as asymptotic climatological c,b values of c = 1.79 and b = 2.13, to which a convergence in the 1950-99 U.S. decadal data is verified.

  17. Hydrologic and climatologic data, 1967, Salt Lake County, Utah

    USGS Publications Warehouse

    Hely, A.G.; Mower, Reed W.; Horr, C.A.

    1968-01-01

    An investigation of the water resources of Salt Lake County, Utah, was undertaken by the Water Resources Division of the U.S. Geological Survey in July 1963. This investigation is a cooperative project financed chiefly by equal contributions of the State of Utah and the Federal Government in accordance with an agreement between the Division of Water Rights, Utah Department of Natural Resources, and the Geological Survey. The investigation was financed during the period covered by this report by the following organizations: Utah Division of Water Rights (formerly State Engineer), Utah Division of Water Resources (formerly Water and Power Board), Salt Lake County, Salt Lake County Water Conservancy District, Central Utah Water Conservancy District, Metropolitan Water District of Salt Lake City, City of Murray, Granger-Hunter Improvement District, Taylorsville-Bennion Improvement District, Holladay Water Company, Magna Water and Sewer District, U.S. Bureau of Reclamation, U.S. Geological Survey.The investigation encompasses the collection and interpretation of a large variety of climatologic, hydrologic, and geologic data in and near Salt Lake County. Utah Basic-Data Releases 11-13 contain data collected through 1966. This release contains climatologic and surfacewater data for the 1967 water year (October 1966 to September 1967) and ground-water data collected during the 1967 calendar year. A similar annual release will contain data collected during the remainder of the investigation, and interpretive reports will be prepared as the investigation proceeds. Organizations that furnished data are acknowledged in station descriptions and footnotes to tables.

  18. Hydrologic and climatologic data, 1968, Salt Lake County, Utah

    USGS Publications Warehouse

    1969-01-01

    An investigation of the water resources of Salt Lake County, Utah, was undertaken by the Water Resources Division of the U.S. Geological Survey in July 1963. This investigation is a cooperative project financed chiefly by equal contributions of the State of Utah and the Federal Government in accordance with an agreement between the Division of Water Rights, Utah Department of Natural Resources, and the Geological Survey. The investigation was financed during the period covered by this report by the following organizations: Utah Division of Water Rights (formerly State Engineer), Utah Division of Water Resources (formerly Water and Power Board), Salt Lake County, Salt Lake County Water Conservancy District, Central Utah Water Conservancy District, Metropolitan Water District of Salt Lake City, City of Murray, Granger-Hunter Improvement District, Taylorsville-Bennion Improvement District, Holladay Water Company, Magna Water and Sewer District, U.S. Bureau of Reclamation, U.S. Geological SurveyThe investigation encompasses the collection and interpretation of a large variety of climatologic, hydrologic, and geologic data in and near Salt Lake County. Utah Basic-Data Releases 11-13 and 15 contain data collected through 1967. This release contains climatologic and surface-water data for the 1968 water year (October 1967 to September 1968) and ground-water data collected during the 1968 calendar year. This is the final annual release of basic data for this investigation. Interpretive reports summarizing the results are in preparation. Organizations that furnished data are acknowledged in station descriptions and footnotes to tables.

  19. The Radiative Forcing Model Intercomparison Project (RFMIP): Experimental protocol for CMIP6

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Pincus, Robert; Forster, Piers M.; Stevens, Bjorn

    The phrasing of the first of three questions motivating CMIP6 – “How does the Earth system respond to forcing?” – suggests that forcing is always well-known, yet the radiative forcing to which this question refers has historically been uncertain in coordinated experiments even as understanding of how best to infer radiative forcing has evolved. The Radiative Forcing Model Intercomparison Project (RFMIP) endorsed by CMIP6 seeks to provide a foundation for answering the question through three related activities: (i) accurate characterization of the effective radiative forcing relative to a near-preindustrial baseline and careful diagnosis of the components of this forcing; (ii) assessment ofmore » the absolute accuracy of clear-sky radiative transfer parameterizations against reference models on the global scales relevant for climate modeling; and (iii) identification of robust model responses to tightly specified aerosol radiative forcing from 1850 to present. Complete characterization of effective radiative forcing can be accomplished with 180 years (Tier 1) of atmosphere-only simulation using a sea-surface temperature and sea ice concentration climatology derived from the host model's preindustrial control simulation. Assessment of parameterization error requires trivial amounts of computation but the development of small amounts of infrastructure: new, spectrally detailed diagnostic output requested as two snapshots at present-day and preindustrial conditions, and results from the model's radiation code applied to specified atmospheric conditions. In conclusion, the search for robust responses to aerosol changes relies on the CMIP6 specification of anthropogenic aerosol properties; models using this specification can contribute to RFMIP with no additional simulation, while those using a full aerosol model are requested to perform at least one and up to four 165-year coupled ocean–atmosphere simulations at Tier 1.« less

  20. The Radiative Forcing Model Intercomparison Project (RFMIP): Experimental protocol for CMIP6

    DOE PAGES

    Pincus, Robert; Forster, Piers M.; Stevens, Bjorn

    2016-09-27

    The phrasing of the first of three questions motivating CMIP6 – “How does the Earth system respond to forcing?” – suggests that forcing is always well-known, yet the radiative forcing to which this question refers has historically been uncertain in coordinated experiments even as understanding of how best to infer radiative forcing has evolved. The Radiative Forcing Model Intercomparison Project (RFMIP) endorsed by CMIP6 seeks to provide a foundation for answering the question through three related activities: (i) accurate characterization of the effective radiative forcing relative to a near-preindustrial baseline and careful diagnosis of the components of this forcing; (ii) assessment ofmore » the absolute accuracy of clear-sky radiative transfer parameterizations against reference models on the global scales relevant for climate modeling; and (iii) identification of robust model responses to tightly specified aerosol radiative forcing from 1850 to present. Complete characterization of effective radiative forcing can be accomplished with 180 years (Tier 1) of atmosphere-only simulation using a sea-surface temperature and sea ice concentration climatology derived from the host model's preindustrial control simulation. Assessment of parameterization error requires trivial amounts of computation but the development of small amounts of infrastructure: new, spectrally detailed diagnostic output requested as two snapshots at present-day and preindustrial conditions, and results from the model's radiation code applied to specified atmospheric conditions. In conclusion, the search for robust responses to aerosol changes relies on the CMIP6 specification of anthropogenic aerosol properties; models using this specification can contribute to RFMIP with no additional simulation, while those using a full aerosol model are requested to perform at least one and up to four 165-year coupled ocean–atmosphere simulations at Tier 1.« less

  1. The East and Southeast Asia Initiatives: Aerosol Column Measurements

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Hsu, Christina N.; Li, Zhanqing

    2003-01-01

    Airborne dusts from northern China contribute a significant part of the air quality problem and, to some extent, regional climatic impact in Asia during spring- time. However, with the economical growth in China, increases in the emission of air pollutants generated from industrial and vehicular sources will not only impact the radiation balance, but adverse health effects to humans all year round. In addition, both of these dust and air pollution clouds can transport swiftly across the Pacific reaching North America within a few days, possessing an even larger scale effect. The Asian dust and air pollution aerosols can be detected by its colored appearance on current Earth observing satellites (e.g., MODIS, SeaWiFS, TOMS, etc.) and its evolution monitored by satellites and surface network. Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially those in Africa, South America, and Southeast Asia. However, the unique climatology of Southeast Asia is very different than that of Africa and South America, such that large-scale biomass burning causes smoke to interact extensively with clouds during the peak-burning season of March to April. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3,Br), and atmospheric aerosols are produced by biomass burning processes. These gases influence the Earth- atmosphere system, impacting both global climate and tropospheric chemistry. Some aerosols can serve as cloud condensation nuclei, which play an important role in determining cloud lifetime and precipitation, hence, altering the earth's radiation and water budget. Biomass burning also affects the biogeochemical cycling of nitrogen and carbon compounds from the soil to the atmosphere; the hydrological cycle (i.e., run off and evaporation); land surface reflectivity and emissivity; as well as ecosystem biodiversity and stability. Two new initiatives, EAST-AIRE (East

  2. TRMM-Based Lightning Climatology

    NASA Technical Reports Server (NTRS)

    Cecil, Daniel J.; Buechler, Dennis E.; Blakeslee, Richard J.

    2011-01-01

    Gridded climatologies of total lightning flash rates seen by the spaceborne Optical Transient Detector (OTD) and Lightning Imaging Sensor (LIS) have been updated. OTD collected data from May 1995 to March 2000. LIS data (equatorward of about 38 deg) has been added for 1998-2010. Flash counts from each instrument are scaled by the best available estimates of detection efficiency. The long LIS record makes the merged climatology most robust in the tropics and subtropics, while the high latitude data is entirely from OTD. The mean global flash rate from the merged climatology is 46 flashes per second. The peak annual flash rate at 0.5 deg scale is 160 fl/square km/yr in eastern Congo. The peak monthly average flash rate at 2.5 scale is 18 fl/square km/mo, from early April to early May in the Brahmaputra Valley of far eastern India. Lightning decreases in this region during the monsoon season, but increases further north and west. A monthly average peak from early August to early September in northern Pakistan also exceeds any monthly averages from Africa, despite central Africa having the greatest yearly average. Most continental regions away from the equator have an annual cycle with lightning flash rates peaking in late spring or summer. The main exceptions are India and southeast Asia, with springtime peaks in April and May. For landmasses near the equator, flash rates peak near the equinoxes. For many oceanic regions, the peak flash rates occur in autumn. This is particularly noticeable for the Mediterranean and North Atlantic. Landmasses have a strong diurnal cycle of lightning, with flash rates generally peaking between 3-5 pm local solar time. The central United States flash rates peak later, in late evening or early night. Flash rates peak after midnight in northern Argentina. These regions are known for large, intense, long-lived mesoscale convective systems.

  3. Easy Volcanic Aerosol

    NASA Astrophysics Data System (ADS)

    Toohey, Matthew; Stevens, Bjorn; Schmidt, Hauke; Timmreck, Claudia

    2016-04-01

    Radiative forcing by stratospheric sulfate aerosol of volcanic origin is one of the strongest drivers of natural climate variability. Transient model simulations attempting to match observed climate variability, such as the CMIP historical simulations, rely on volcanic forcing reconstructions based on observations of a small sample of recent eruptions and coarse proxy data for eruptions before the satellite era. Volcanic forcing data sets used in CMIP5 were provided either in terms of optical properties, or in terms of sulfate aerosol mass, leading to significant inter-model spread in the actual volcanic radiative forcing produced by models and in their resulting climate responses. It remains therefore unclear to what degree inter-model spread in response to volcanic forcing represents model differences or variations in the forcing. In order to isolate model differences, Easy Volcanic Aerosol (EVA) provides an analytic representation of volcanic stratospheric aerosol forcing, based on available observations and aerosol model results, prescribing the aerosol's radiative properties and primary modes of spatial and temporal variability. In contrast to regriddings of observational data, EVA allows for the production of physically consistent forcing for historic and hypothetical eruptions of varying magnitude, source latitude, and season. Within CMIP6, EVA will be used to reconstruct volcanic forcing over the past 2000 years for use in the Paleo-Modeling Intercomparison Project (PMIP), and will provide forcing sets for VolMIP experiments aiming to quantify model uncertainty in the response to volcanic forcing. Here, the functional form of EVA will be introduced, along with illustrative examples including the EVA-based reconstruction of volcanic forcing over the historical period, and that of the 1815 Tambora eruption.

  4. Spatiotemporal variability and contribution of different aerosol types to the Aerosol Optical Depth over the Eastern Mediterranean.

    PubMed

    Georgoulias, Aristeidis K; Alexandri, Georgia; Kourtidis, Konstantinos A; Lelieveld, Jos; Zanis, Prodromos; Pöschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2016-01-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the Aerosol Optical Depth (AOD) over the Eastern Mediterranean as derived from MODIS Terra (3/2000-12/2012) and Aqua (7/2002-12/2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sunphotometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium sized cities, industrial zones, and power plant complexes, seasonal variabilities, and decadal averages. The average AOD at 550 nm (AOD 550 ) for the entire region is ~ 0.22 ± 0.19 with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in Central and Eastern Europe, and transport of dust from the Sahara Desert and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD 550 . The spatial and temporal variability of anthropogenic, dust and fine mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD 550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine mode natural aerosols account for ~ 51 %, ~ 34 % and ~ 15 % of the total AOD 550 over land, while, anthropogenic aerosols, dust and marine aerosols account ~ 40 %, ~ 34 % and ~ 26 % of the total AOD 550 over the sea, based on MODIS Terra and Aqua observations.

  5. The role of global cloud climatologies in validating numerical models

    NASA Technical Reports Server (NTRS)

    HARSHVARDHAN

    1991-01-01

    The net upward longwave surface radiation is exceedingly difficult to measure from space. A hybrid method using General Circulation Model (GCM) simulations and satellite data from the Earth Radiation Budget Experiment (ERBE) and the International Satellite Cloud Climatology Project (ISCCP) was used to produce global maps of this quantity over oceanic areas. An advantage of this technique is that no independent knowledge or assumptions regarding cloud cover for a particular month are required. The only information required is a relationship between the cloud radiation forcing (CRF) at the top of the atmosphere and that at the surface, which is obtained from the GCM simulation. A flow diagram of the technique and results are given.

  6. Development of Modal Aerosol Module in CAM5 for Biogeochemical Cycles

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Liu, Xiaohong

    2017-11-18

    This project aims at developing new capabilities for the Modal Aerosol Module in the DOE’s E3SM model with the applications to the global biogeochemical cycle. The impacts of the new developments on model simulations of clouds and climate will be examined. There are thee objectives for this project study: Implementing primary marine organic aerosols into the modal aerosol module (MAM) and investigate effects of primary marine organic aerosols on climate in E3SM; Implementing dust speciation in MAM and investigate the effect of dust species on mixed-phase clouds through indirect effects in E3SM; Writing papers documenting the new MAM developments (e.g.,more » MAM4 documentation paper, marine organic aerosol paper, dust speciation); These objectives will be accomplished in collaborations with Drs. Phil Rasch, Steve Ghan, and Susannah Burrows at Pacific Northwest National Laboratory.« less

  7. Air pollution from gas flaring: new emission factor estimates and detection in a West African aerosol remote-sensing climatology

    NASA Astrophysics Data System (ADS)

    MacKenzie, Rob; Fawole, Olusegun Gabriel; Levine, James; Cai, Xiaoming

    2016-04-01

    Gas flaring, the disposal of gas through stacks in an open-air flame, is a common feature in the processing of crude oil, especially in oil-rich regions of the world. Gas flaring is a prominent source of volatile organic compounds (VOCs), polycyclic aromatic hydrocarbons (PAH), CO, CO2, nitrogen oxides (NOx), SO2 (in "sour" gas only), and soot (black carbon), as well as the release of locally significant amounts of heat. The rates of emission of these pollutants from gas flaring depend on a number of factors including, but not limited to, fuel composition and quantity, stack geometry, flame/combustion characteristics, and prevailing meteorological conditions. Here, we derive new estimated emission factors (EFs) for carbon-containing pollutants (excluding PAH). The air pollution dispersion model, ADMS5, is used to simulate the dispersion of the pollutants from flaring stacks in the Niger delta. A seasonal variation of the dispersion pattern of the pollutant within a year is studied in relation to the movements of the West Africa Monsoon (WAM) and other prevailing meteorological factors. Further, we have clustered AERONET aerosol signals using trajectory analysis to identify dominant aerosol sources at the Ilorin site in West Africa (4.34 oE, 8.32 oN). A 10-year trajectory-based analysis was undertaken (2005-2015, excluding 2010). Of particular interest are air masses that have passed through the gas flaring region in the Niger Delta area en-route the AERONET site. 7-day back trajectories were calculated using the UK Universities Global Atmospheric Modelling Programme (UGAMP) trajectory model which is driven by analyses from the European Centre for Medium-Range Weather Forecasts (ECMWF). From the back-trajectory calculations, dominant sources are identified, using literature classifications: desert dust (DD); Biomass burning (BB); and Urban-Industrial (UI). We use a combination of synoptic trajectories and aerosol optical properties to distinguish a fourth source

  8. Intercomparison of aerosol-cloud-precipitation interactions in stratiform orographic mixed-phase clouds

    NASA Astrophysics Data System (ADS)

    Muhlbauer, A.; Hashino, T.; Xue, L.; Teller, A.; Lohmann, U.; Rasmussen, R. M.; Geresdi, I.; Pan, Z.

    2010-04-01

    . Furthermore, it is found that neither a decrease in cloud droplet coalescence nor a decrease in riming necessarily implies a decrease in precipitation due to compensation effects by other microphysical pathways. The simulations suggest that mixed-phase conditions play an important role in reducing the overall susceptibility of clouds and precipitation with respect to changes in the aerosols number concentrations. As a consequence the indirect aerosol effect on precipitation is suggested to be less pronounced or even inverted in regions with high terrain (e.g., the Alps or Rocky Mountains) or in regions where mixed-phase microphysics climatologically plays an important role for orographic precipitation.

  9. Does Aerosol Geoengineering the Earth's Climate Pass a Cost-Benefit Test?

    NASA Astrophysics Data System (ADS)

    Keller, K.; Urban, N.; Tuana, N.

    2007-12-01

    Anthropogenic carbon dioxide (CO2) emissions are changing the Earth's climate with potentially dangerous consequences. Ratified international agreements call for a reduction of CO2 emissions to avoid dangerous anthropogenic interference with the climate system. Recent studies have, however, proposed an alternative strategy: to geoengineer Earth's climate by injecting aerosol precursors into the stratosphere. It is often claimed that aerosol geoengineering would provide net economic benefits because geoengineering requires far lower near-term investments compared to deep cuts in CO2 emissions. However, aerosol geoengineering projects can also cause nontrivial economic costs. This is because aerosol geoengineering hinges on successfully counterbalancing the forcing effects of CO2 emissions (which decay over centuries) with the forcing effects of aerosol emissions (which decay within years). A failure to maintain this delicate balance can lead to abrupt climatic changes, with potentially substantial economic damages. Deferring cuts in CO2 emissions in favor of aerosol geoengineering is hence a deeply uncertain gamble, as it requires so far unknown institutions to reliably control aerosol forcings over centuries. Here we use a simple economic model to evaluate potential costs and benefits of aerosol geoengineering for a wide range of the deeply uncertain parameters. We show that aerosol geoengineering projects may cause economic damages that can far exceed the benefits and may hence fail a cost-benefit test.

  10. The SPARC Intercomparison of Middle Atmosphere Climatologies

    NASA Technical Reports Server (NTRS)

    Randel, William; Fleming, Eric; Geller, Marvin; Gelman, Mel; Hamilton, Kevin; Karoly, David; Ortland, Dave; Pawson, Steve; Swinbank, Richard; Udelhofen, Petra

    2003-01-01

    Our current confidence in 'observed' climatological winds and temperatures in the middle atmosphere (over altitudes approx. 10-80 km) is assessed by detailed intercomparisons of contemporary and historic data sets. These data sets include global meteorological analyses and assimilations, climatologies derived from research satellite measurements, and historical reference atmosphere circulation statistics. We also include comparisons with historical rocketsonde wind and temperature data, and with more recent lidar temperature measurements. The comparisons focus on a few basic circulation statistics, such as temperature, zonal wind, and eddy flux statistics. Special attention is focused on tropical winds and temperatures, where large differences exist among separate analyses. Assimilated data sets provide the most realistic tropical variability, but substantial differences exist among current schemes.

  11. Characterizing Aerosol Distributions and Optical Properties Using the NASA Langley High Spectral Resolution Lidar

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hostetler, Chris; Ferrare, Richard

    The objective of this project was to provide vertically and horizontally resolved data on aerosol optical properties to assess and ultimately improve how models represent these aerosol properties and their impacts on atmospheric radiation. The approach was to deploy the NASA Langley Airborne High Spectral Resolution Lidar (HSRL) and other synergistic remote sensors on DOE Atmospheric Science Research (ASR) sponsored airborne field campaigns and synergistic field campaigns sponsored by other agencies to remotely measure aerosol backscattering, extinction, and optical thickness profiles. Synergistic sensors included a nadir-viewing digital camera for context imagery, and, later in the project, the NASA Goddard Institutemore » for Space Studies (GISS) Research Scanning Polarimeter (RSP). The information from the remote sensing instruments was used to map the horizontal and vertical distribution of aerosol properties and type. The retrieved lidar parameters include profiles of aerosol extinction, backscatter, depolarization, and optical depth. Products produced in subsequent analyses included aerosol mixed layer height, aerosol type, and the partition of aerosol optical depth by type. The lidar products provided vertical context for in situ and remote sensing measurements from other airborne and ground-based platforms employed in the field campaigns and was used to assess the predictions of transport models. Also, the measurements provide a data base for future evaluation of techniques to combine active (lidar) and passive (polarimeter) measurements in advanced retrieval schemes to remotely characterize aerosol microphysical properties. The project was initiated as a 3-year project starting 1 January 2005. It was later awarded continuation funding for another 3 years (i.e., through 31 December 2010) followed by a 1-year no-cost extension (through 31 December 2011). This project supported logistical and flight costs of the NASA sensors on a dedicated aircraft, the

  12. A New Paradigm for Diagnosing Contributions to Model Aerosol Forcing Error: Diagnosing Model Aerosol Forcing Error

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Jones, A. L.; Feldman, D. R.; Freidenreich, S.

    A new paradigm in benchmark absorption-scattering radiative transfer is presented that enables both the globally averaged and spatially resolved testing of climate model radiation parameterizations in order to uncover persistent sources of biases in the aerosol instantaneous radiative effect (IRE). A proof of concept is demonstrated with the Geophysical Fluid Dynamics Laboratory AM4 and Community Earth System Model 1.2.2 climate models. Instead of prescribing atmospheric conditions and aerosols, as in prior intercomparisons, native snapshots of the atmospheric state and aerosol optical properties from the participating models are used as inputs to an accurate radiation solver to uncover model-relevant biases. Thesemore » diagnostic results show that the models' aerosol IRE bias is of the same magnitude as the persistent range cited (~1 W/m 2) and also varies spatially and with intrinsic aerosol optical properties. The findings presented here underscore the significance of native model error analysis and its dispositive ability to diagnose global biases, confirming its fundamental value for the Radiative Forcing Model Intercomparison Project.« less

  13. A New Paradigm for Diagnosing Contributions to Model Aerosol Forcing Error: Diagnosing Model Aerosol Forcing Error

    DOE PAGES

    Jones, A. L.; Feldman, D. R.; Freidenreich, S.; ...

    2017-12-07

    A new paradigm in benchmark absorption-scattering radiative transfer is presented that enables both the globally averaged and spatially resolved testing of climate model radiation parameterizations in order to uncover persistent sources of biases in the aerosol instantaneous radiative effect (IRE). A proof of concept is demonstrated with the Geophysical Fluid Dynamics Laboratory AM4 and Community Earth System Model 1.2.2 climate models. Instead of prescribing atmospheric conditions and aerosols, as in prior intercomparisons, native snapshots of the atmospheric state and aerosol optical properties from the participating models are used as inputs to an accurate radiation solver to uncover model-relevant biases. Thesemore » diagnostic results show that the models' aerosol IRE bias is of the same magnitude as the persistent range cited (~1 W/m 2) and also varies spatially and with intrinsic aerosol optical properties. The findings presented here underscore the significance of native model error analysis and its dispositive ability to diagnose global biases, confirming its fundamental value for the Radiative Forcing Model Intercomparison Project.« less

  14. A Global Solar Irradiance Climatology of an Intermountain Region.

    DTIC Science & Technology

    1986-01-01

    D-A!171 97 A GLOBAL SOLAIR IRRRDIANCE CLIMATOLOGY OF AN INTERMOUNTAIN REGION(U) AIR FORCE INST OF TECH MRIGHT-PATTERSON APR ON E W DOBRY 1986...DD~ I JAN 73 1473 EDITION OF I NOV 65 IS OBSOLETE SECURITY CLASSIFICATION OF THIS PAGE Denfata E1ilered) %.ir.. , t . ~. ~ ~ ~ $~:V ( e vis ABSTRACT...Professor: Dr. G. E . Bingham De artment: Soil Science and Biometeorology A global solar irradiance climatology of an intermountain region is developed using

  15. Jupiter Climatological Database from Frequent 5-25 µm Mid-IR Spectral Mapping using IRTF/TEXES

    NASA Astrophysics Data System (ADS)

    Fletcher, Leigh N.; Orton, Glenn S.; Greathouse, Thomas K.; Sinclair, James; Irwin, Patrick G. J.; Giles, Rohini S.; Encrenaz, Therese; Drossart, Pierre

    2015-11-01

    We report on the development of a long-term Jovian Climatological Database (JCliD) to explore variability in Jupiter’s atmospheric temperatures, winds, clouds and composition- from long-term seasonal changes to short-term major upheavals. Radiometrically calibrated spectral scan maps of Jupiter have been regularly obtained using the TEXES instrument (Texas Echelon cross Echelle Spectrograph, Lacy et al. 2002, PASP 114, p153-168) between 2012 and 2015. Ten settings between 5 and 25 µm (10-20 cm-1 wide settings at spectral resolutions of 2000-10000) were selected to be sensitive to jovian temperatures (via H2, CH4 and CH3D), tropospheric phosphine and ammonia, tropospheric haze opacity and stratospheric hydrocarbons ethane and acetylene. Diffraction-limited spatial resolutions of 0.6-1.6” were achieved. Observations over consecutive nights allow the creation of full spatial maps for comparison with the visible light record, revealing ephemeral stratospheric wave activity, NEB hotspots, heating at the northern auroral oval, and complex thermal signatures associated with tropospheric vortices, waves and barges. Full spectra are inverted via the NEMESIS retrieval algorithm (Irwin et al., 2008, JSQRT 109, p1136-1150) to map temperatures at multiple altitudes (1-600 mbar), winds, aerosol opacity and gaseous composition. The spatial and spectral resolutions of the resulting maps surpass those obtained during the Cassini flyby of Jupiter in 2000, and permit temporal interpolation to understand the environmental conditions related to the emergence and evolution of discrete features. In December 2014 we find warmer temperatures in the northern stratosphere (a seasonal effect in late northern summer despite Jupiter’s small axial tilt); a hemispheric asymmetry in the tropospheric PH3 distribution due to variations in the vigour of vertical mixing and photolytic shielding; elevated PH3, aerosols and NH3 in the equatorial zone (EZ) related to equatorial uplift; elevated

  16. MERIS albedo climatology and its effect on the FRESCO+ O2 A-band cloud retrieval from SCIAMACHY data

    NASA Astrophysics Data System (ADS)

    Popp, Christoph; Wang, Ping; Brunner, Dominik; Stammes, Piet; Zhou, Yipin

    2010-05-01

    Accurate cloud information is an important prerequisite for the retrieval of atmospheric trace gases from spaceborne UV/VIS sensors. Errors in the estimated cloud fraction and cloud height (pressure) result in an erroneous air mass factor and thus can lead to inaccuracies in the vertical column densities of the retrieved trace gas. In ESA's TEMIS (Tropospheric Emission Monitoring Internet Service) project, the FRESCO+ (Fast Retrieval Scheme for Clouds from the Oxygen A-band) cloud retrieval is applied to, amongst others, SCIAMACHY (SCanning Imaging Absorption SpectroMeter for Atmospheric CartograpHY) data to determine these quantities. Effective cloud fraction and pressure are inverted by (i) radiative transfer simulations of top-of-atmosphere reflectance based on O2 absorption, single Rayleigh scattering, surface and cloud albedo in three spectral windows covering the O2 A-band and (ii) a subsequent fitting of the simulated to the measured spectrum. However, FRESCO+ relies on a relatively coarse resolution surface albedo climatology (1° x 1°) compiled from GOME (Global Ozone Monitoring Experiment) measurements in the 1990's which introduces several artifacts, e.g. an overestimation of cloud fraction at coastlines or over some mountainous regions. Therefore, we test the substitution of the GOME climatology with a new land surface albedo climatology compiled for every month from MEdium Resolution Imaging Spectrometer (MERIS) Albedomap data (0.05° x 0.05°) covering the period January 2003 to October 2006. The MERIS channels at 754nm and 775nm are located spectrally close to the corresponding GOME channels (758nm and 772nm) on both sides of the O2 A-band. Further, the increased spatial resolution of the MERIS product allows to better account for SCIAMACHY's pixel size of approximately 30x60km. The aim of this study is to describe and assess (i) the compilation and quality of the MERIS climatology (ii) the differences to the GOME climatology, and (iii) possible

  17. Competing influences of greenhouse warming and aerosols on Asian summer monsoon circulation and rainfall

    NASA Astrophysics Data System (ADS)

    Lau, William Ka-Ming; Kim, Kyu-Myong

    2017-05-01

    In this paper, we have compared and contrasted competing influences of greenhouse gases (GHG) warming and aerosol forcing on Asian summer monsoon circulation and rainfall based on CMIP5 historical simulations. Under GHG-only forcing, the land warms much faster than the ocean, magnifying the pre-industrial climatological land-ocean thermal contrast and hemispheric asymmetry, i.e., warmer northern than southern hemisphere. A steady increasing warm-ocean-warmer-land (WOWL) trend has been in effect since the 1950's substantially increasing moisture transport from adjacent oceans, and enhancing rainfall over the Asian monsoon regions. However, under GHG warming, increased atmospheric stability due to strong reduction in mid-tropospheric and near surface relative humidity coupled to an expanding subsidence areas, associated with the Deep Tropical Squeeze (DTS, Lau and Kim, 2015b) strongly suppress monsoon convection and rainfall over subtropical and extratropical land, leading to a weakening of the Asian monsoon meridional circulation. Increased anthropogenic aerosol emission strongly masks WOWL, by over 60% over the northern hemisphere, negating to a large extent the rainfall increase due to GHG warming, and leading to a further weakening of the monsoon circulation, through increasing atmospheric stability, most likely associated with aerosol solar dimming and semi-direct effects. Overall, we find that GHG exerts stronger positive rainfall sensitivity, but less negative circulation sensitivity in SASM compared to EASM. In contrast, aerosols exert stronger negative impacts on rainfall, but less negative impacts on circulation in EASM compared to SASM.

  18. Climate Implications of the Heterogeneity of Anthropogenic Aerosol Forcing

    NASA Astrophysics Data System (ADS)

    Persad, Geeta Gayatri

    ' surface versus atmospheric forcing. Future aerosol emissions patterns will affect the distribution of regional climate impacts. This dissertation interrogates how international trade affects existing assumptions about East Asia's future black carbon aerosol emissions, using integrated assessment modeling, emissions and economic data, and AM3 simulations. Exports emerge as a uniquely large and potentially growing source of Chinese black carbon emissions that could impede projected regional emissions reductions, with substantial climate and health consequences. The findings encourage greater emissions projection sophistication and illustrate how societal decisions may influence future aerosol forcing heterogeneity.

  19. Cavity Ring-Down Measurement of Aerosol Optical Properties During the Asian Dust Above Monterey Experiment and DOE Aerosol Intensive Operating Period

    NASA Technical Reports Server (NTRS)

    Ricci, K.; Strawa, A. W.; Provencal, R.; Castaneda, R.; Bucholtz, A.; Schmid, B.

    2004-01-01

    Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300/Mm with an estimated precision of 0.1/Mm for 1550 nm light and 0.2/Mm for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects. We present comparisons between the Cadenza measurements and those from a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS 14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

  20. Cavity Ring-Down Measurement of Aerosol Optical Properties During the Asian Dust Above Monterey Experiment and DOE Aerosol Intensive Operating Period

    NASA Astrophysics Data System (ADS)

    Ricci, K.; Strawa, A. W.; Provencal, R.; Castaneda, R.; Bucholtz, A.; Schmid, B.

    2003-12-01

    Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300 Mm-1 with an estimated precision of 0.1 Mm-1 for 1550 nm light and 0.2 Mm-1 for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects. We present comparisons between the Cadenza measurements and those from a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

  1. Identification and climatology of cut-off lows near the tropopause.

    PubMed

    Nieto, R; Sprenger, M; Wernli, H; Trigo, R M; Gimeno, L

    2008-12-01

    Cut-off low pressure systems (COLs) are defined as closed lows in the upper troposphere that have become completely detached from the main westerly current. These slow-moving systems often affect the weather conditions at the earth's surface and also work as a mechanism of mass transfer between the stratosphere and the troposphere, playing a significant role in the net flow of tropospheric ozone. In the first part of this work we provide a comprehensive summary of results obtained in previous studies of COLs. Following this, we present three long-term climatologies of COLs. The first two climatologies are based on the conceptual model of a COL, using European Centre for Medium-range Weather Forecasts (ECMWF) analyses (1958-2002) and National Centers for Environmental Prediction-National Center for Atmospheric Research (1948-2006) reanalysis data sets. The third climatology uses a different method of detection, which is based on using potential vorticity as the physical parameter of diagnosis. This approach was applied only to the ECMWF reanalysis data. The final part of the paper is devoted to comparing results obtained by these different climatologies in terms of areas of preferential occurrence, life span, and seasonal cycle. Despite some key differences, the three climatologies agree in terms of the main areas of COL occurrence, namely (1) southwestern Europe, (2) the eastern north Pacific coast, and (3) the north China-Siberian region. However, it is also shown that the detection of these areas of main COL occurrence, as obtained using the potential vorticity approach, depends on the level of isentropic analysis used.

  2. Nine-year spatial and temporal evolution of desert dust aerosols over South and East Asia as revealed by CALIOP

    NASA Astrophysics Data System (ADS)

    Proestakis, Emmanouil; Amiridis, Vassilis; Marinou, Eleni; Georgoulias, Aristeidis K.; Solomos, Stavros; Kazadzis, Stelios; Chimot, Julien; Che, Huizheng; Alexandri, Georgia; Binietoglou, Ioannis; Daskalopoulou, Vasiliki; Kourtidis, Konstantinos A.; de Leeuw, Gerrit; van der A, Ronald J.

    2018-02-01

    We present a 3-D climatology of the desert dust distribution over South and East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network). The method involves the use of the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, applied to multiyear CALIPSO observations (January 2007-December 2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over South and East Asia along with the seasonal transition of dust transport pathways. Persistent high D_AOD (dust aerosol optical depth) values at 532 nm, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with the highest values observed during spring for northern China (Taklimakan and Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally, we decompose the CALIPSO AOD (aerosol optical depth) into dust and non-dust aerosol components to reveal the non-dust AOD over the highly industrialized and densely populated regions of South and East Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D_AOD time series and trends between January 2007 and December 2015 are calculated over South and East Asia and over selected subregions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China trends are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.

  3. Modelling absorbing aerosol with ECHAM-HAM: Insights from regional studies

    NASA Astrophysics Data System (ADS)

    Tegen, Ina; Heinold, Bernd; Schepanski, Kerstin; Banks, Jamie; Kubin, Anne; Schacht, Jacob

    2017-04-01

    Quantifying distributions and properties of absorbing aerosol is a basis for investigations of interactions of aerosol particles with radiation and climate. While evaluations of aerosol models by field measurements can be particularly successful at the regional scale, such results need to be put into a global context for climate studies. We present an overview over studies performed at the Leibniz Institute for Tropospheric Research aiming at constraining the properties of mineral dust and soot aerosol in the global aerosol model ECHAM6-HAM2 based on different regional studies. An example is the impact of different sources for dust transported to central Asia, which is influenced, by far-range transport of dust from Arabia and the Sahara together with dust from local sources. Dust types from these different source regions were investigated in the context of the CADEX project and are expected to have different optical properties. For Saharan dust, satellite retrievals from MSG SEVIRI are used to constrain Saharan dust sources and optical properties. In the Arctic region, on one hand dust aerosol is simulated in the framework of the PalMod project. On the other hand aerosol measurements that will be taken during the DFG-funded (AC)3 field campaigns will be used to evaluate the simulated transport pathways of soot aerosol from European, North American and Asian sources, as well as the parameterization of soot ageing processes in ECHAM6-HAM2. Ultimately, results from these studies will improve the representation of aerosol absorption in the global model.

  4. Future changes in the climatology of the Great Plains low-level jet derived from fine resolution multi-model simulations

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Tang, Ying; Winkler, Julie; Zhong, Shiyuan

    The southerly Great Plains low-level jet (GPLLJ) is one of the most significant circulation features of the central U.S. linking large-scale atmospheric circulation with the regional climate. GPLLJs transport heat and moisture, contribute to thunderstorm and severe weather formation, provide a corridor for the springtime migration of birds and insects, enhance wind energy availability, and disperse air pollution. We also assess future changes in GPLLJ frequency using an eight member ensemble of dynamically-downscaled climate simulations for the mid-21st century. Nocturnal GPLLJ frequency is projected to increase in the southern plains in spring and in the central plains in summer, whereasmore » current climatological patterns persist into the future for daytime and cool season GPLLJs. The relationship between future GPLLJ frequency and the extent and strength of anticyclonic airflow over eastern North America varies with season. Most simulations project a westward shift of anticyclonic airflow in summer, but uncertainty is larger for spring with only half of the simulations suggesting a westward expansion. Furthemore, the choice of regional climate model and the driving lateral boundary conditions have a large influence on the projected future changes in GPLLJ frequency and highlight the importance of multi-model ensembles to estimate the uncertainty surrounding the future GPLLJ climatology.« less

  5. Future changes in the climatology of the Great Plains low-level jet derived from fine resolution multi-model simulations.

    PubMed

    Tang, Ying; Winkler, Julie; Zhong, Shiyuan; Bian, Xindi; Doubler, Dana; Yu, Lejiang; Walters, Claudia

    2017-07-10

    The southerly Great Plains low-level jet (GPLLJ) is one of the most significant circulation features of the central U.S. linking large-scale atmospheric circulation with the regional climate. GPLLJs transport heat and moisture, contribute to thunderstorm and severe weather formation, provide a corridor for the springtime migration of birds and insects, enhance wind energy availability, and disperse air pollution. We assess future changes in GPLLJ frequency using an eight member ensemble of dynamically-downscaled climate simulations for the mid-21st century. Nocturnal GPLLJ frequency is projected to increase in the southern plains in spring and in the central plains in summer, whereas current climatological patterns persist into the future for daytime and cool season GPLLJs. The relationship between future GPLLJ frequency and the extent and strength of anticyclonic airflow over eastern North America varies with season. Most simulations project a westward shift of anticyclonic airflow in summer, but uncertainty is larger for spring with only half of the simulations suggesting a westward expansion. The choice of regional climate model and the driving lateral boundary conditions have a large influence on the projected future changes in GPLLJ frequency and highlight the importance of multi-model ensembles to estimate the uncertainty surrounding the future GPLLJ climatology.

  6. Future changes in the climatology of the Great Plains low-level jet derived from fine resolution multi-model simulations

    DOE PAGES

    Tang, Ying; Winkler, Julie; Zhong, Shiyuan; ...

    2017-07-10

    The southerly Great Plains low-level jet (GPLLJ) is one of the most significant circulation features of the central U.S. linking large-scale atmospheric circulation with the regional climate. GPLLJs transport heat and moisture, contribute to thunderstorm and severe weather formation, provide a corridor for the springtime migration of birds and insects, enhance wind energy availability, and disperse air pollution. We also assess future changes in GPLLJ frequency using an eight member ensemble of dynamically-downscaled climate simulations for the mid-21st century. Nocturnal GPLLJ frequency is projected to increase in the southern plains in spring and in the central plains in summer, whereasmore » current climatological patterns persist into the future for daytime and cool season GPLLJs. The relationship between future GPLLJ frequency and the extent and strength of anticyclonic airflow over eastern North America varies with season. Most simulations project a westward shift of anticyclonic airflow in summer, but uncertainty is larger for spring with only half of the simulations suggesting a westward expansion. Furthemore, the choice of regional climate model and the driving lateral boundary conditions have a large influence on the projected future changes in GPLLJ frequency and highlight the importance of multi-model ensembles to estimate the uncertainty surrounding the future GPLLJ climatology.« less

  7. A Total Ozone Dependent Ozone Profile Climatology Based on Ozone-Sondes and Aura MLS Data

    NASA Astrophysics Data System (ADS)

    Labow, G. J.; McPeters, R. D.; Ziemke, J. R.

    2014-12-01

    A new total ozone-based ozone profile climatology has been created for use in satellite and/or ground based ozone retrievals. This climatology was formed by combining data from the Microwave Limb Sounder (MLS) with data from balloon sondes and binned by zone and total ozone. Because profile shape varies with total column ozone, this climatology better captures the ozone variations than the previously used seasonal climatologies, especially near the tropopause. This is significantly different than ozone climatologies used in the past as there is no time component. The MLS instrument on Aura has excellent latitude coverage and measures ozone profiles daily from the upper troposphere to the lower mesosphere at ~3.5 km resolution. Almost a million individual MLS ozone measurements are merged with data from over 55,000 ozonesondes which are then binned as a function of total ozone. The climatology consists of average ozone profiles as a function of total ozone for six 30 degree latitude bands covering altitudes from 0-75 km (in Z* pressure altitude coordinates). This new climatology better represents the profile shape as a function of total ozone than previous climatologies and shows some remarkable and somewhat unexpected correlations between total ozone and ozone in the lower altitudes, particularly in the lower and middle troposphere. These data can also be used to infer biases and errors in either the MLS retrievals or ozone sondes.

  8. Long-term changes of aerosol optical and radiative properties and their role in global dimming and brightening

    NASA Astrophysics Data System (ADS)

    Hatzianastassiou, N.; Papadimas, C. D.; Matsoukas, C.; Pavlakis, K.; Fotiadi, A.; Wild, M.; Vardavas, I.

    2009-04-01

    Global dimming and brightening (GDB) have profound effects on the Earth's environment. For example, GDB counteracts or supplements greenhouse warming. Atmospheric aerosols, through their interaction with solar radiation (direct, indirect and semi-direct effects) can affect GDB. Changes in aerosol burden or other physical and optical properties can modify tendencies of GDB. For example, satellite observations of aerosol amounts, available since the early 1980s, but only over the oceans, indicate a downward trend since about 1990, consistent with the observed brightening during this period. There is a need, however, to investigate similar trends, but also over land, and to relate them with contemporary GDB. The seasonal and inter-annual variability of the natural, but also anthropogenic aerosol direct radiative effect on solar radiation at the Earth's surface (DREsurf) and the contribution of aerosols to global dimming and brightening (GDB) is estimated over the period 1984-2001. This is achieved by using a spectral radiative transfer model together with Total Ozone Mapping Spectrometer (TOMS) aerosol optical thickness (AOT) and other satellite (International Satellite Cloud Climatology Project, ISCCP-D2), NCEP/NCAR reanalysis and Global Aerosol Data Set (GADS) data for surface and atmospheric parameters. The major findings are mostly related to natural and less to anthropogenic aerosols because of limitations of the TOMS observational technique. The model results indicate that aerosols exert a strong surface cooling over the globe by reducing locally the incoming surface solar radiation by up to 70 W m-2. This direct radiative effect averaged over the globe for the period 1984-2001, is equivalent to 5 W m-2, associated with 6.5 and 3.5 W m-2, for the Northern and Southern Hemispheres, respectively. However, this aerosol DREsurf effect shows an important inter-annual variability as large as 200%. A strong solar brightening, or decreased aerosol DREsurf, by as much as

  9. The impacts of aerosol loading, composition, and water uptake on aerosol extinction variability in the Baltimore-Washington, D.C. region

    NASA Astrophysics Data System (ADS)

    Beyersdorf, A. J.; Ziemba, L. D.; Chen, G.; Corr, C. A.; Crawford, J. H.; Diskin, G. S.; Moore, R. H.; Thornhill, K. L.; Winstead, E. L.; Anderson, B. E.

    2016-01-01

    In order to utilize satellite-based aerosol measurements for the determination of air quality, the relationship between aerosol optical properties (wavelength-dependent, column-integrated extinction measured by satellites) and mass measurements of aerosol loading (PM2.5 used for air quality monitoring) must be understood. This connection varies with many factors including those specific to the aerosol type - such as composition, size, and hygroscopicity - and to the surrounding atmosphere, such as temperature, relative humidity (RH), and altitude, all of which can vary spatially and temporally. During the DISCOVER-AQ (Deriving Information on Surface conditions from Column and Vertically Resolved Observations Relevant to Air Quality) project, extensive in situ atmospheric profiling in the Baltimore, MD-Washington, D.C. region was performed during 14 flights in July 2011. Identical flight plans and profile locations throughout the project provide meaningful statistics for determining the variability in and correlations between aerosol loading, composition, optical properties, and meteorological conditions. Measured water-soluble aerosol mass was composed primarily of ammonium sulfate (campaign average of 32 %) and organics (57 %). A distinct difference in composition was observed, with high-loading days having a proportionally larger percentage of sulfate due to transport from the Ohio River Valley. This composition shift caused a change in the aerosol water-uptake potential (hygroscopicity) such that higher relative contributions of inorganics increased the bulk aerosol hygroscopicity. These days also tended to have higher relative humidity, causing an increase in the water content of the aerosol. Conversely, low-aerosol-loading days had lower sulfate and higher black carbon contributions, causing lower single-scattering albedos (SSAs). The average black carbon concentrations were 240 ng m-3 in the lowest 1 km, decreasing to 35 ng m-3 in the free troposphere (above

  10. Long-term observations of aerosol and cloud condensation nuclei concentrations in Barbados

    NASA Astrophysics Data System (ADS)

    Pöhlker, Mira L.; Klimach, Thomas; Krüger, Ovid O.; Hrabe de Angelis, Isabella; Ditas, Florian; Praß, Maria; Holanda, Bruna; Su, Hang; Weber, Bettina; Pöhlker, Christopher; Farrell, David A.; Stevens, Bjorn; Prospero, Joseph M.; Andreae, Meinrat O.; Pöschl, Ulrich

    2017-04-01

    Long-term observation of atmospheric aerosol and cloud condensation nuclei (CCN) concentrations has been conducted at the Ragged Point site in Barbados since August 2016. Ragged Point is a well-established station to monitor the transatlantic transport of Saharan dust outbreaks [1]. In the absence of dust plumes, it represents an ideal site to analyze the maritime boundary layer aerosol that is transported with the trade winds over the Atlantic towards Barbados [2,3]. Broad aerosol size distribution (10 nm to 10 µm) as well as size-resolved CCN measurements at 10 different supersaturations from 0.05 % to 0.84 % have been conducted. The continuous online analyses are supplemented by intensive sampling periods to probe specific aerosol properties with various offline techniques (i.e., microscopy and spectroscopy). Aerosol key properties from our measurements are compared with the continuous and in depth observation of cloud properties at Deebles Point, which is in close neighborhood to the Ragged Point site [2]. Moreover, our activities have been synchronized with the HALO-NARVAL-2 aircraft campaign in August 2016 that added further detailed information on shallow cumulus clouds, which are characteristic for the Atlantic trade winds and represent a crucial factor in the Earth climate system. Our measurements have the following two focal points: (i) We aim to obtain a detailed CCN climatology for the alternation of maritime and dust-impacted episodes at this unique coastal location. This study will complement our recent in-depth analysis for the long-term CCN variability at a remote rain forest location [4]. (ii) Furthermore, we aim to collect detailed information on the role of different aerosol populations on the properties of the climatically important shallow cumulus clouds. References: [1] Prospero, J. M., Collard, F. X., Molinie, J., Jeannot, A. (2014), Global Biogeochemical Cycles, 28, 757-773. [2] Stevens, B., et al. (2016), Bulletin of the American

  11. Role of absorbing aerosols on hot extremes in India in a GCM

    NASA Astrophysics Data System (ADS)

    Mondal, A.; Sah, N.; Venkataraman, C.; Patil, N.

    2017-12-01

    Temperature extremes and heat waves in North-Central India during the summer months of March through June are known for causing significant impact in terms of human health, productivity and mortality. While greenhouse gas-induced global warming is generally believed to intensify the magnitude and frequency of such extremes, aerosols are usually associated with an overall cooling, by virtue of their dominant radiation scattering nature, in most world regions. Recently, large-scale atmospheric conditions leading to heat wave and extreme temperature conditions have been analysed for the North-Central Indian region. However, the role of absorbing aerosols, including black carbon and dust, is still not well understood, in mediating hot extremes in the region. In this study, we use 30-year simulations from a chemistry-coupled atmosphere-only General Circulation Model (GCM), ECHAM6-HAM2, forced with evolving aerosol emissions in an interactive aerosol module, along with observed sea surface temperatures, to examine large-scale and mesoscale conditions during hot extremes in India. The model is first validated with observed gridded temperature and reanalysis data, and is found to represent observed variations in temperature in the North-Central region and concurrent large-scale atmospheric conditions during high temperature extremes realistically. During these extreme events, changes in near surface properties include a reduction in single scattering albedo and enhancement in short-wave solar heating rate, compared to climatological conditions. This is accompanied by positive anomalies of black carbon and dust aerosol optical depths. We conclude that the large-scale atmospheric conditions such as the presence of anticyclones and clear skies, conducive to heat waves and high temperature extremes, are exacerbated by absorbing aerosols in North-Central India. Future air quality regulations are expected to reduce sulfate particles and their masking of GHG warming. It is

  12. Reconciling the aerosol-liquid water path relationship in the ECHAM6-HAM GCM and the Aerosol_cci/Cloud_cci (A)ATSR dataset by minimizing the effect of aerosol swelling

    NASA Astrophysics Data System (ADS)

    Neubauer, D.; Christensen, M.; Lohmann, U.; Poulsen, C. A.

    2016-12-01

    Studies using present day variability to assess statistical relationships between aerosol and cloud properties find different strengths of these relationships between satellite data and general circulation model (GCM) data. This discrepancy can be explained by structural uncertainties due to differences in the analysis/observational scale and the process scale or spurious relationships between aerosol and cloud properties. Such spurious relationships are the growth of aerosol particles in the humid environment surrounding clouds, misclassification of partly cloudy satellite pixels as cloud free pixels, brightening of aerosol particles by sunlight reflected at cloud edges, or effects of clouds on aerosol like processing of aerosol particles in clouds by nucleation or impact scavenging and subsequent growth by heterogeneous chemistry and release by cloud droplet evaporation or wet scavenging of aerosol particles. To minimize the effects of spatial aggregation and spurious relationships we apply a new nearest neighbour approach to high resolution (A)ATSR datasets from the Aerosol_cci and Cloud_cci projects of the Climate Change Initiative (CCI) programme of ESA. For the ECHAM6-HAM GCM we quantify the impact of using dry aerosol (without aerosol water) in the analysis to mimic the effect of the nearest neighbour approach. The aerosol-liquid water path relationship in ECHAM6-HAM is systematically stronger than in (A)ATSR data and cannot be explained by an overestimation of autoconversion when using diagnostic precipitation but rather by aerosol swelling in regions where humidity is high and clouds are present. When aerosol water is removed from the analysis in ECHAM6-HAM the strength of the aerosol-liquid water path relationship agrees much better with the ones of (A)ATSR or MODIS. We further find that while the observed relationships of different satellite sensors ((A)ATSR vs. MODIS) are not always consistent for tested environmental conditions the relationships in

  13. Climatology and trends of aerosol optical depth over the Mediterranean basin during the last 12years (2002-2014) based on Collection 006 MODIS-Aqua data.

    PubMed

    Floutsi, A A; Korras-Carraca, M B; Matsoukas, C; Hatzianastassiou, N; Biskos, G

    2016-05-01

    The Mediterranean basin is a region of particular interest for studying atmospheric aerosols due to the large variety of air masses it receives, and its sensitivity to climate change. In this study we use the newest collection (C006) of aerosol optical depth from MODIS-Aqua, from which we also derived the fine-mode fraction and Ångström exponent over the last 12years (i.e., from 2002 to 2014), providing the longest analyzed dataset for this region. The long-term regional optical depth average is 0.20±0.05, with the indicated uncertainty reflecting the inter-annual variability. Overall, the aerosol optical depth exhibits a south-to-north decreasing gradient and an average decreasing trend of 0.0030 per year (19% total decrease over the study period). The correlation between the reported AOD observations with measurements from the ground AERONET stations is high (R=0.76-0.80 depending on the wavelength), with the MODIS-Aqua data being slightly overestimated. Both fine-fraction and Ångström exponent data highlight the dominance of anthropogenic aerosols over the northern, and of desert aerosols over the southern part of the region. Clear intrusions of desert dust over the Eastern Mediterranean are observed principally in spring, and in some cases in winter. Dust intrusions dominate the Western Mediterranean in the summer (and sometimes in autumn), whereas anthropogenic aerosols dominate the sub-region of the Black Sea in all seasons but especially during summer. Fine-mode optical depth is found to decrease over almost all areas of the study region during the 12-year period, marking the decreasing contribution of anthropogenic particulate matter emissions over the study area. Coarse-mode aerosol load also exhibits an overall decreasing trend. However, its decrease is smaller than that of fine aerosols and not as uniformly distributed, underlining that the overall decrease in the region arises mainly from reduced anthropogenic emissions. Copyright © 2016 Elsevier

  14. Aerosol cloud interactions in southeast Pacific stratocumulus: satellite observations, in situ data and regional modeling

    NASA Astrophysics Data System (ADS)

    George, Rhea

    The influence of anthropogenic aerosols on cloud radiative properties in the persistent southeast Pacific stratocumulus deck is investigated using MODIS satellite observations, in situ data from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx), and WRF-Chem, a regional model with interactive chemistry and aerosols. An albedo proxy is derived based on the fractional coverage of low cloud (a macrophysical field) and the cloud albedo, with the latter broken down into contributions from microphysics (cloud droplet concentration, Nd and macrophysics (liquid water path). Albedo variability is dominated by low cloud fraction variability, except within 10-15° of the South American coast, where cloud albedo variability contributes significantly. Covariance between cloud fraction and cloud albedo also contributes significantly to the variance in albedo, which highlights how complex and inseparable the factors controlling albedo are. N d variability contributes only weakly, which emphasizes that attributing albedo variability to the indirect effects of aerosols against the backdrop of natural meteorological variability is extremely challenging. Specific cases of aerosol changes can have strong impacts on albedo. We identify a pathway for periodic anthropogenic aerosol transport to the unpolluted marine stratocumulus >1000 km offshore, which strongly enhances Nd and albedo in zonally-elongated 'hook'-shaped arc. Hook development occurs with Nd increasing to polluted levels over the remote ocean primarily due to entrainment of a large number of small aerosols from the free troposphere that contribute a relatively small amount of aerosol mass to the marine boundary layer. Strong, deep offshore flow needed to transport continental aerosols to the remote ocean is favored by a trough approaching the South American coast and a southeastward shift of the climatological subtropical high pressure system. DMS significantly influences the aerosol number and

  15. The Regional Environmental Impacts of Atmospheric Aerosols over Egypt

    NASA Astrophysics Data System (ADS)

    Zakey, Ashraf; Ibrahim, Alaa

    2015-04-01

    due to airborne particles washed out by rain events. Conversely, the AOD increases in summer because particle accumulation is favored by the absence of precipitation during this season. Moreover, in summer, photochemical processes in the atmosphere lead to slight increases in the values of aerosol optical characteristics, despite lower wind speeds [hence less wind-blown dust] relative to other seasons. This study has been conducted under the PEER 2-239 research project titled "the Impact of Biogenic and Anthropogenic Atmospheric Aerosols to Climate in Egypt". Project website: CleanAirEgypt.org

  16. The regime of biomass burning aerosols over the Mediterranean basin based on satellite observations

    NASA Astrophysics Data System (ADS)

    Kalaitzi, Nikoleta; Gkikas, Antonis; Papadimas, Christos. D.; Hatzianastassiou, Nikolaos; Torres, Omar; Mihalopoulos, Nikolaos

    2016-04-01

    specifically, the algorithm examines the fulfillment of these criteria for Ångström Exponent (AE), Fine Fraction (FF) and Aerosol Index (AI). The AE and FF data, which are characteristic of the aerosol size, are derived from multispectralCollection 006 MODIS-AquaAerosol Optical Depth (AOD) data, whereas the AI data, that characterize the absorption ability of aerosols, are taken from the OMI-Aura database. The algorithm enables the identification of BB aerosols over specific geographical cells (pixels) throughout the study region, over both sea and land surfaces, during days of the 2005-2015 period. The results make possible the construction of a climatological-like database of Mediterranean BB aerosols, permitting to perceive the geographical patterns of their regime, namely the areas in which they occur, in relation to their timing, i.e. the months and seasons of their occurrence. This regime is quantified, which means that the frequency (absolute and percent) of occurrence of BB aerosols is calculated, along with the associated computed AOD values. The year by year variability of BB aerosols is also investigated over the period 2005-2015, with emphasis to inter-annual and seasonal tendencies.

  17. Climatology of salt transitions and implications for stone weathering.

    PubMed

    Grossi, C M; Brimblecombe, P; Menéndez, B; Benavente, D; Harris, I; Déqué, M

    2011-06-01

    This work introduces the notion of salt climatology. It shows how climate affects salt thermodynamic and the potential to relate long-term salt damage to climate types. It mainly focuses on specific sites in Western Europe, which include some cities in France and Peninsular Spain. Salt damage was parameterised using the number of dissolution-crystallisation events for unhydrated (sodium chloride) and hydrated (sodium sulphate) systems. These phase transitions have been calculated using daily temperature and relative humidity from observation meteorological data and Climate Change models' output (HadCM3 and ARPEGE). Comparing the number of transitions with meteorological seasonal data allowed us to develop techniques to estimate the frequency of salt transitions based on the local climatology. Results show that it is possible to associate the Köppen-Geiger climate types with potential salt weathering. Temperate fully humid climates seem to offer the highest potential for salt damage and possible higher number of transitions in summer. Climates with dry summers tend to show a lesser frequency of transitions in summer. The analysis of temperature, precipitation and relative output from Climate Change models suggests changes in the Köppen-Geiger climate types and changes in the patterns of salt damage. For instance, West Europe areas with a fully humid climate may change to a more Mediterranean like or dry climates, and consequently the seasonality of different salt transitions. The accuracy and reliability of the projections might be improved by simultaneously running multiple climate models (ensembles). Copyright © 2011 Elsevier B.V. All rights reserved.

  18. Climatologies at high resolution for the earth’s land surface areas

    PubMed Central

    Karger, Dirk Nikolaus; Conrad, Olaf; Böhner, Jürgen; Kawohl, Tobias; Kreft, Holger; Soria-Auza, Rodrigo Wilber; Zimmermann, Niklaus E.; Linder, H. Peter; Kessler, Michael

    2017-01-01

    High-resolution information on climatic conditions is essential to many applications in environmental and ecological sciences. Here we present the CHELSA (Climatologies at high resolution for the earth’s land surface areas) data of downscaled model output temperature and precipitation estimates of the ERA-Interim climatic reanalysis to a high resolution of 30 arc sec. The temperature algorithm is based on statistical downscaling of atmospheric temperatures. The precipitation algorithm incorporates orographic predictors including wind fields, valley exposition, and boundary layer height, with a subsequent bias correction. The resulting data consist of a monthly temperature and precipitation climatology for the years 1979–2013. We compare the data derived from the CHELSA algorithm with other standard gridded products and station data from the Global Historical Climate Network. We compare the performance of the new climatologies in species distribution modelling and show that we can increase the accuracy of species range predictions. We further show that CHELSA climatological data has a similar accuracy as other products for temperature, but that its predictions of precipitation patterns are better. PMID:28872642

  19. Multi-year downscaling application of two-way coupled WRF v3.4 and CMAQ v5.0.2 over east Asia for regional climate and air quality modeling: model evaluation and aerosol direct effects

    NASA Astrophysics Data System (ADS)

    Hong, Chaopeng; Zhang, Qiang; Zhang, Yang; Tang, Youhua; Tong, Daniel; He, Kebin

    2017-06-01

    In this study, a regional coupled climate-chemistry modeling system using the dynamical downscaling technique was established by linking the global Community Earth System Model (CESM) and the regional two-way coupled Weather Research and Forecasting - Community Multi-scale Air Quality (WRF-CMAQ) model for the purpose of comprehensive assessments of regional climate change and air quality and their interactions within one modeling framework. The modeling system was applied over east Asia for a multi-year climatological application during 2006-2010, driven with CESM downscaling data under Representative Concentration Pathways 4.5 (RCP4.5), along with a short-term air quality application in representative months in 2013 that was driven with a reanalysis dataset. A comprehensive model evaluation was conducted against observations from surface networks and satellite observations to assess the model's performance. This study presents the first application and evaluation of the two-way coupled WRF-CMAQ model for climatological simulations using the dynamical downscaling technique. The model was able to satisfactorily predict major meteorological variables. The improved statistical performance for the 2 m temperature (T2) in this study (with a mean bias of -0.6 °C) compared with the Coupled Model Intercomparison Project Phase 5 (CMIP5) multi-models might be related to the use of the regional model WRF and the bias-correction technique applied for CESM downscaling. The model showed good ability to predict PM2. 5 in winter (with a normalized mean bias (NMB) of 6.4 % in 2013) and O3 in summer (with an NMB of 18.2 % in 2013) in terms of statistical performance and spatial distributions. Compared with global models that tend to underpredict PM2. 5 concentrations in China, WRF-CMAQ was able to capture the high PM2. 5 concentrations in urban areas. In general, the two-way coupled WRF-CMAQ model performed well for both climatological and air quality applications. The coupled

  20. Aerosol Microphysics and Radiation Integration

    DTIC Science & Technology

    2003-09-30

    656-4769 email: reidj@nrlmry.navy.mil Award Number: N0001403WX20570 http://www.nrlmry.navy.mil/aerosol/ http://www.nrlmry.navy.mil/ flambe ...Fire Locating and Modeling of Burning Emissions ( FLAMBE ) project, which also provides NAAPS with a real-time biomass burning source function. In...Locating and Modeling of Burning Emissions ( FLAMBE ) project are currently being utilized by internet community, Air quality/human health research

  1. Spatiotemporal variability and contribution of different aerosol types to the Aerosol Optical Depth over the Eastern Mediterranean

    PubMed Central

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos A.; Lelieveld, Jos; Zanis, Prodromos; Pöschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2018-01-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the Aerosol Optical Depth (AOD) over the Eastern Mediterranean as derived from MODIS Terra (3/2000–12/2012) and Aqua (7/2002–12/2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sunphotometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium sized cities, industrial zones, and power plant complexes, seasonal variabilities, and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is ~ 0.22 ± 0.19 with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in Central and Eastern Europe, and transport of dust from the Sahara Desert and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine mode natural aerosols account for ~ 51 %, ~ 34 % and ~ 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account ~ 40 %, ~ 34 % and ~ 26 % of the total AOD550 over the sea, based on MODIS Terra and Aqua observations. PMID:29755508

  2. Spatiotemporal variability and contribution of different aerosol types to the aerosol optical depth over the Eastern Mediterranean

    NASA Astrophysics Data System (ADS)

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos A.; Lelieveld, Jos; Zanis, Prodromos; Pöschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2016-11-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the aerosol optical depth (AOD) over the Eastern Mediterranean as derived from MODIS (Moderate Resolution Imaging Spectroradiometer) Terra (March 2000-December 2012) and Aqua (July 2002-December 2012) satellite instruments. For this purpose, a 0.1° × 0.1° gridded MODIS dataset was compiled and validated against sun photometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium-sized cities, industrial zones and power plant complexes, seasonal variabilities and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is ˜ 0.22 ± 0.19, with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in central and eastern Europe and transport of dust from the Sahara and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine-mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine-mode natural aerosols account for ˜ 51, ˜ 34 and ˜ 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account ˜ 40, ˜ 34 and ˜ 26 % of the total AOD550 over the sea, based on

  3. Spatiotemporal Variability and Contribution of Different Aerosol Types to the Aerosol Optical Depth over the Eastern Mediterranean

    NASA Technical Reports Server (NTRS)

    Georgoulias, Aristeidis K.; Alexandri, Georgia; Kourtidis, Konstantinos A.; Lelieveld, Jos; Zanis, Prodromos; Poeschl, Ulrich; Levy, Robert; Amiridis, Vassilis; Marinou, Eleni; Tsikerdekis, Athanasios

    2016-01-01

    This study characterizes the spatiotemporal variability and relative contribution of different types of aerosols to the aerosol optical depth (AOD) over the Eastern Mediterranean as derived from MODIS (Moderate Resolution Imaging Spectroradiometer) Terra (March 2000-December 2012) and Aqua (July 2002-December 2012) satellite instruments. For this purpose, a 0.1deg × 0.1deg gridded MODIS dataset was compiled and validated against sun photometric observations from the AErosol RObotic NETwork (AERONET). The high spatial resolution and long temporal coverage of the dataset allows for the determination of local hot spots like megacities, medium-sized cities, industrial zones and power plant complexes, seasonal variabilities and decadal averages. The average AOD at 550 nm (AOD550) for the entire region is approx. 0.22 +/- 0.19, with maximum values in summer and seasonal variabilities that can be attributed to precipitation, photochemical production of secondary organic aerosols, transport of pollution and smoke from biomass burning in central and eastern Europe and transport of dust from the Sahara and the Middle East. The MODIS data were analyzed together with data from other satellite sensors, reanalysis projects and a chemistry-aerosol-transport model using an optimized algorithm tailored for the region and capable of estimating the contribution of different aerosol types to the total AOD550. The spatial and temporal variability of anthropogenic, dust and fine-mode natural aerosols over land and anthropogenic, dust and marine aerosols over the sea is examined. The relative contribution of the different aerosol types to the total AOD550 exhibits a low/high seasonal variability over land/sea areas, respectively. Overall, anthropogenic aerosols, dust and fine-mode natural aerosols account for approx. 51, approx. 34 and approx. 15 % of the total AOD550 over land, while, anthropogenic aerosols, dust and marine aerosols account approx. 40, approx. 34 and approx. 26 % of

  4. Spatial and Temporal Monitoring of Aerosol over Selected Urban Areas in Egypt

    NASA Astrophysics Data System (ADS)

    Shokr, Mohammed; El-Tahan, Mohammed; Ibrahim, Alaa

    2015-04-01

    We utilize remote sensing data of atmospheric aerosols from the Moderate Resolution Imaging Spectroradiometer (MODIS) aboard the Terra and Aqua satellites to explore spatio-temporal patterns over selected urban sites in Egypt during 2000-2015. High resolution (10 x 10 km^2) Level 2, collection 5, quality-controlled product was used. The selected sites are characterized by different human and industrial activities as well as landscape and meteorological attributes. These have impacts on the dominant types and intensity of aerosols. Aerosol robotic network (AERONET) data were used to validate the calculations from MODIS. The suitability of the MODIS product in terms of spatial and temporal coverage as well as accuracy and robustness has been established. Seasonal patterns of aerosol concentration are identified and compared between the sites. Spatial gradient of aerosol is assessed in the vicinity of major aerosol-emission sites (e.g. Cairo) to determine the range of influence of the generated pollution. Peak aerosol concentrations are explained in terms of meteorological events and land cover. The limited trends found in the temporal records of the aerosol measurements will be confirmed using calibrated long-term ground observations. The study has been conducted under the PEER 2-239 research project titled "The Impact of Biogenic and Anthropogenic Atmospheric Aerosols to Climate in Egypt". Project website is CleanAirEgypt.org

  5. Aerosol-associated changes in tropical stratospheric ozone following the eruption of Mount Pinatubo

    NASA Technical Reports Server (NTRS)

    Grant, William B.; Browell, Edward V.; Fishman, Jack; Brackett, Vincent G.; Veiga, Robert E.; Nganga, Dominique; Minga, A.; Cros, Bernard; Butler, Carolyn F.; Fenn, Marta A.

    1994-01-01

    The large amount of sulfuric acid aerosol formed in the stratosphere by conversion of sulfur dioxide emitted by the eruption of Mount Pinatubo (15.14 deg N, 120.35 deg E) in the Philippines around June 15, 1991, has had a pronounced effect on lower stratospheric ozone in the tropics. Measurements of stratospheric ozone in the tropics using electrochemical concentration cell (ECC) sondes before and after the eruption and the airborne UV differential absorption lidar (DIAL) system after the eruption are compared with Stratospheric Aerosol and Gas Experiment II (SAGE II) measurements from several years before the eruption and ECC sonde measurements from the year prior to the eruption to determine the resulting changes. Ozone decreases of up to 33 % compared with SAGE II climatological values were found to be directly correlated with altitude regions of enhanced aerosol loading in the 16- to 28-km range. A maximum partial-column decrease of 29 +/- Dobson units (DU) was found over the 16- to 28-km range in September 1991 along with small increases (to 5.9 +/- 2 DU) from 28 to 31.5 km. A large decrease of ozone was also found at 4 deg to 8 deg S from May to August 1992, with a maximum decrease of 33 +/- 7 DU found above Brazzaville in July. Aerosol data form the visible channel of the advanced very high resolution radiometer (AVHRR) and the visible wavelength of the UV DIAL system were used to examine the relationship between aerosol (surface area) densities and ozone changes. The tropical stratospheric ozone changes we observed in 1991 and 1992 are likely be explained by a combination of dynamical (vertical transport) perturbations, radiative perturbations on ozone photochemistry, and heterogeneous chemistry.

  6. Weather Conditions During the 2013 SAS/SOAS Field Campaign: Providing Meteorological Context to the Extensive Project Measurements

    NASA Astrophysics Data System (ADS)

    Moore, J.; Farkas, C. M.

    2013-12-01

    The Southeast Atmosphere Study (SAS)/Southern Oxidant and Aerosol Study (SOAS) (url: http://www.eol.ucar.edu/projects/sas/) was a joint project supported by the National Science Foundation, the Environmental Protection Agency, Electric Power Research Institute and 30 US and International Research Institutions, and was the largest U.S. air quality study in decades. This collaborative project addressed various components of air quality, chemical and aerosol constituent evolution over the SE US. An international team of investigators brought an unprecedented suite of chemical species filter sampling equipment and in-situ sensors to characterize the atmosphere and the chemical processes occurring within it with specific emphasis on the characterization of the content, form and evolution of chemical and aerosol species in the humid Southeast US from 1 June-15 July during summer. The main ';super site' brought ~100 participants and ~50 specialized samplers and analyzers to the EPRI sponsored SouthEastern Aerosol and Atmospheric Characterization (SEARCH) Network site near Brent, Alabama. The purpose of this presentation is to provide the meteorological context to the observations that were made at the central Alabama ';super site' described above. The long-term climatology of the region suggested that the weather would be relatively quiet during the period with the occasional air mass change (frontal passage) and a few days of showers and/or windy conditions. What actually happened during the 45-day campaign was generally a much more unsettled period that included several frontal passages, a large number of rainy days and cooler than normal temperatures. Table 1 provides a preliminary summary of conditions during the campaign. The number of quiet or stagnant periods that might allow the buildup of various chemical constituents important to the study were infrequent and did not last for extended periods. Contact will be made with the Alabama State Climatologist to improve

  7. Aerosol climate time series from ESA Aerosol_cci (Invited)

    NASA Astrophysics Data System (ADS)

    Holzer-Popp, T.

    2013-12-01

    Within the ESA Climate Change Initiative (CCI) the Aerosol_cci project (mid 2010 - mid 2013, phase 2 proposed 2014-2016) has conducted intensive work to improve algorithms for the retrieval of aerosol information from European sensors AATSR (3 algorithms), PARASOL, MERIS (3 algorithms), synergetic AATSR/SCIAMACHY, OMI and GOMOS. Whereas OMI and GOMOS were used to derive absorbing aerosol index and stratospheric extinction profiles, respectively, Aerosol Optical Depth (AOD) and Angstrom coefficient were retrieved from the other sensors. Global datasets for 2008 were produced and validated versus independent ground-based data and other satellite data sets (MODIS, MISR). An additional 17-year dataset is currently generated using ATSR-2/AATSR data. During the three years of the project, intensive collaborative efforts were made to improve the retrieval algorithms focusing on the most critical modules. The team agreed on the use of a common definition for the aerosol optical properties. Cloud masking was evaluated, but a rigorous analysis with a pre-scribed cloud mask did not lead to improvement for all algorithms. Better results were obtained using a post-processing step in which sudden transitions, indicative of possible occurrence of cloud contamination, were removed. Surface parameterization, which is most critical for the nadir only algorithms (MERIS and synergetic AATSR / SCIAMACHY) was studied to a limited extent. The retrieval results for AOD, Ångström exponent (AE) and uncertainties were evaluated by comparison with data from AERONET (and a limited amount of MAN) sun photometer and with satellite data available from MODIS and MISR. Both level2 and level3 (gridded daily) datasets were validated. Several validation metrics were used (standard statistical quantities such as bias, rmse, Pearson correlation, linear regression, as well as scoring approaches to quantitatively evaluate the spatial and temporal correlations against AERONET), and in some cases

  8. Implementation of aerosol-cloud interactions in the regional atmosphere-aerosol model COSMO-MUSCAT(5.0) and evaluation using satellite data

    NASA Astrophysics Data System (ADS)

    Dipu, Sudhakar; Quaas, Johannes; Wolke, Ralf; Stoll, Jens; Mühlbauer, Andreas; Sourdeval, Odran; Salzmann, Marc; Heinold, Bernd; Tegen, Ina

    2017-06-01

    The regional atmospheric model Consortium for Small-scale Modeling (COSMO) coupled to the Multi-Scale Chemistry Aerosol Transport model (MUSCAT) is extended in this work to represent aerosol-cloud interactions. Previously, only one-way interactions (scavenging of aerosol and in-cloud chemistry) and aerosol-radiation interactions were included in this model. The new version allows for a microphysical aerosol effect on clouds. For this, we use the optional two-moment cloud microphysical scheme in COSMO and the online-computed aerosol information for cloud condensation nuclei concentrations (Cccn), replacing the constant Cccn profile. In the radiation scheme, we have implemented a droplet-size-dependent cloud optical depth, allowing now for aerosol-cloud-radiation interactions. To evaluate the models with satellite data, the Cloud Feedback Model Intercomparison Project Observation Simulator Package (COSP) has been implemented. A case study has been carried out to understand the effects of the modifications, where the modified modeling system is applied over the European domain with a horizontal resolution of 0.25° × 0.25°. To reduce the complexity in aerosol-cloud interactions, only warm-phase clouds are considered. We found that the online-coupled aerosol introduces significant changes for some cloud microphysical properties. The cloud effective radius shows an increase of 9.5 %, and the cloud droplet number concentration is reduced by 21.5 %.

  9. Biomass-Burning Aerosols in South East-Asia: Smoke Impact Assessment (BASE-ASIA)

    NASA Technical Reports Server (NTRS)

    Tsay, S.-C.; Hsu, N. C.; King, M. D.; Sun, W.-Y.

    2004-01-01

    Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially those in Africa, South America, and Southeast Asia. However, the unique climatology of Southeast Asia is very different than that of Africa and South America, such that large-scale biomass burning causes smoke to interact extensively with clouds during the peak-burning season of March to April. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass burning processes. These gases influence the Earth- atmosphere system, impacting both global climate and tropospheric chemistry. Some aerosols can serve as cloud condensation nuclei, which play an important role in determining cloud lifetime and precipitation, hence, altering the earth s radiation and water budget. Analyses from satellite measurements reveal the reflected solar (emitted thermal) radiation from clouds due to smoke aerosols can be reduced (enhanced) by 100 (20) Watts per square meter over the month of March 2000. In addition, the reduction in cloud spectral reflectance is large enough to lead to significant errors in satellite retrievals of cloud properties (e.g., optical thickness and effective radius). The fresh water distribution in this region is highly dependent on monsoon rainfall; in fact, the predictability of the tropical climate system is much reduced during the boreal spring. Therefore, to accurately assess the impact of smoke aerosols in this region requires continuous observations from satellites, aircraft, ground-based networks and dedicated field experiments. BASE-ASIA initiative has been proposed and will be discussed.

  10. Aerosol Optical Properties in Southeast Asia From AERONET Observations

    NASA Astrophysics Data System (ADS)

    Eck, T. F.; Holben, B. N.; Boonjawat, J.; Le, H. V.; Schafer, J. S.; Reid, J. S.; Dubovik, O.; Smirnov, A.

    2003-12-01

    There is little published data available on measured optical properties of aerosols in the Southeast Asian region. The AERONET project and collaborators commenced monitoring of aerosol optical properties in February 2003 at four sites in Thailand and two sites in Viet Nam to measure the primarily anthropogenic aerosols generated by biomass burning and fossil fuel combustion/ industrial emissions. Automatic sun/sky radiometers at each site measured spectral aerosol optical depth in 7 wavelengths from 340 to 1020 nm and combined with directional radiances in the almucantar, retrievals were made of spectral single scattering albedo and aerosol size distributions. Angstrom exponents, size distributions and spectral single scattering albedo of primarily biomass burning aerosols at rural sites are compared to measurements made at AERONET sites in other major biomass burning regions in tropical southern Africa, South America, and in boreal forest regions. Additionally, the aerosol single scattering albedo and size distributions measured in Bangkok, Thailand are compared with those measured at other urban sites globally. The influences of aerosols originating from other regions outside of Southeast Asia are analyzed using trajectory analyses. Specifically, cases of aerosol transport and mixing from Southern China and from India are presented.

  11. Aerosol and monsoon climate interactions over Asia

    NASA Astrophysics Data System (ADS)

    Li, Zhanqing; Lau, W. K.-M.; Ramanathan, V.; Wu, G.; Ding, Y.; Manoj, M. G.; Liu, J.; Qian, Y.; Li, J.; Zhou, T.; Fan, J.; Rosenfeld, D.; Ming, Y.; Wang, Y.; Huang, J.; Wang, B.; Xu, X.; Lee, S.-S.; Cribb, M.; Zhang, F.; Yang, X.; Zhao, C.; Takemura, T.; Wang, K.; Xia, X.; Yin, Y.; Zhang, H.; Guo, J.; Zhai, P. M.; Sugimoto, N.; Babu, S. S.; Brasseur, G. P.

    2016-12-01

    biomass burning, and biogenic aerosols from vegetation are considered integral components of an intrinsic aerosol-monsoon climate system, subject to external forcing of global warming, anthropogenic aerosols, and land use and change. Future research on aerosol-monsoon interactions calls for an integrated approach and international collaborations based on long-term sustained observations, process measurements, and improved models, as well as using observations to constrain model simulations and projections.

  12. Secondary Aerosol Formation over the ESCOMPTE Area: Results from airborne Aerosol and Trace Gas Measurements

    NASA Astrophysics Data System (ADS)

    van Dingenen, R.; Martins-Dos Santos, S.; Putaud, J. P.; Allet, C.; Bretton, E.; Perros, P.

    2003-04-01

    From June 10th to July 14th 2001, the ESCOMPTE campaign took place in the Marseille-Berre area in Southern France. The goal of the campaign was to produce a high quality 3-D data base from emissions, transport and air composition measurements during urban photochemical pollution episodes at the meso-scale. The CAATER AEROPLUM project was embedded within this international field campaign. AEROPLUM aimed at mapping size distributions of aerosols and photo-oxidants in the mixed layer over the ESCOMPTE domain, using the ARAT Fokker 27 as measurement platform. Aircraft sub-micrometer aerosol measurements are validated during overpasses against ground-based measurements, carried out with similar instrumentation. We will present and discuss data during periods of seabreeze, transporting coastal industrial and urban pollution land-inwards. This leads to intense photochemical activity, evidenced by elevated O_3 concentrations and aerosol levels.

  13. Climate Impacts of CALIPSO-Guided Corrections to Black Carbon Aerosol Vertical Distributions in a Global Climate Model

    NASA Astrophysics Data System (ADS)

    Kovilakam, Mahesh; Mahajan, Salil; Saravanan, R.; Chang, Ping

    2017-10-01

    We alleviate the bias in the tropospheric vertical distribution of black carbon aerosols (BC) in the Community Atmosphere Model (CAM4) using the Cloud-Aerosol and Infrared Pathfinder Satellite Observations (CALIPSO)-derived vertical profiles. A suite of sensitivity experiments are conducted with 1x, 5x, and 10x the present-day model estimated BC concentration climatology, with (corrected, CC) and without (uncorrected, UC) CALIPSO-corrected BC vertical distribution. The globally averaged top of the atmosphere radiative flux perturbation of CC experiments is ˜8-50% smaller compared to uncorrected (UC) BC experiments largely due to an increase in low-level clouds. The global average surface temperature increases, the global average precipitation decreases, and the ITCZ moves northward with the increase in BC radiative forcing, irrespective of the vertical distribution of BC. Further, tropical expansion metrics for the poleward extent of the Northern Hemisphere Hadley cell (HC) indicate that simulated HC expansion is not sensitive to existing model biases in BC vertical distribution.

  14. The optical properties, physical properties and direct radiative forcing of urban columnar aerosols in the Yangtze River Delta, China

    NASA Astrophysics Data System (ADS)

    Zhuang, Bingliang; Wang, Tijian; Liu, Jane; Che, Huizheng; Han, Yong; Fu, Yu; Li, Shu; Xie, Min; Li, Mengmeng; Chen, Pulong; Chen, Huimin; Yang, Xiu-qun; Sun, Jianning

    2018-02-01

    The optical and physical properties as well as the direct radiative forcings (DRFs) of fractionated aerosols in the urban area of the western Yangtze River Delta (YRD) are investigated with measurements from a Cimel sun photometer combined with a radiation transfer model. Ground-based observations of aerosols have much higher temporal resolutions than satellite retrievals. An initial analysis reveals the characteristics of the optical properties of different types of fractionated aerosols in the western YRD. The total aerosols, mostly composed of scattering components (93.8 %), have mean optical depths of 0.65 at 550 nm and refractive index of 1.44 + 0.0084i at 440 nm. The fine aerosols are approximately four times more abundant and have very different compositions from coarse aerosols. The absorbing components account for only ˜ 4.6 % of fine aerosols and 15.5 % of coarse aerosols and have smaller sizes than the scattering aerosols within the same mode. Therefore, fine particles have stronger scattering than coarse ones, simultaneously reflecting the different size distributions between the absorbing and scattering aerosols. The relationships among the optical properties quantify the aerosol mixing and imply that approximately 15 and 27.5 % of the total occurrences result in dust- and black-carbon-dominating mixing aerosols, respectively, in the western YRD. Unlike the optical properties, the size distributions of aerosols in the western YRD are similar to those found at other sites over eastern China on a climatological scale, peaking at radii of 0.148 and 2.94 µm. However, further analysis reveals that the coarse-dominated particles can also lead to severe haze pollution over the YRD. Observation-based estimations indicate that both fine and coarse aerosols in the western YRD exert negative DRFs, and this is especially true for fine aerosols (-11.17 W m-2 at the top of atmosphere, TOA). A higher absorption fraction leads directly to the negative DRF being

  15. Regional Aerosol Forcing over India: Preliminary Results from the South West Asian Aerosol-Monsoon Interactions (SWAAMI) Aircraft Experiment

    NASA Astrophysics Data System (ADS)

    Morgan, W.; Brooks, J.; Fox, C.; Haslett, S.; Liu, D.; Kompalli, S. K.; Pathak, H.; Manoj, M. R.; Allan, J. D.; Haywood, J. M.; Highwood, E.; Langridge, J.; Nanjundaiah, R. S.; Krishnamoorthy, K.; Babu, S. S.; Satheesh, S. K.; Turner, A. G.; Coe, H.

    2016-12-01

    Aerosol particles from multiple sources across the Indian subcontinent build up to form a dense and extensive haze across the region in advance of the monsoon. These aerosols are thought to perturb the regional radiative balance and hydrological cycle, which may have a significant impact on the monsoon circulation, as well as influencing the associated cloud and rainfall of the system. However the nature and magnitude of such impacts are poorly understood or constrained. Major uncertainties relevant to the regional aerosol burden include its vertical distribution, the relative contribution of different pollution sources and natural emissions and the role of absorbing aerosol species (black carbon and mineral dust). The South West Asian Aerosol-Monsoon Interactions (SWAAMI) project sought to address these major uncertainties by conducting an airborne experiment during June/July 2016 on-board the UK Facility for Airborne Atmospheric Measurement (FAAM) BAe-146 research aircraft. Based out of Lucknow in the), The aircraft conducted multiple flights from Lucknow in the heart of the Indo-Gangetic Plain (IGP) in advance of the monsoon and during the onset phase. The spatial and vertical distribution of aerosol was evaluated across northern India, encompassing drier desert-like regions to the west, heavily populated urban and industrial centres over the IGP and air masses in outflow regions to the south-east towards the Bay of Bengal. Principal measurements included aerosol chemical composition using an Aerodyne Aerosol Mass Spectrometer and a DMT Single Particle Soot Photometer, alongside a Leosphere backscatter LIDAR. Sulphate was a major contributor to the aerosol burden across India, while the organic aerosol was elevated and more dominant over the most polluted regions of the IGP. Substantial aerosol concentrations were frequently observed up to altitudes of approximately 6km, with notable changes in aerosol chemical and physical properties when comparing different

  16. Combined Retrievals of Boreal Forest Fire Aerosol Properties with a Polarimeter and Lidar

    NASA Technical Reports Server (NTRS)

    Knobelspiesse, K.; Cairns, B.; Ottaviani, M.; Ferrare, R.; Haire, J.; Hostetler, C.; Obland, M.; Rogers, R.; Redemann, J.; Shinozuka, Y.; hide

    2011-01-01

    Absorbing aerosols play an important, but uncertain, role in the global climate. Much of this uncertainty is due to a lack of adequate aerosol measurements. While great strides have been made in observational capability in the previous years and decades, it has become increasingly apparent that this development must continue. Scanning polarimeters have been designed to help resolve this issue by making accurate, multi-spectral, multi-angle polarized observations. This work involves the use of the Research Scanning Polarimeter (RSP). The RSP was designed as the airborne prototype for the Aerosol Polarimetery Sensor (APS), which was due to be launched as part of the (ultimately failed) NASA Glory mission. Field observations with the RSP, however, have established that simultaneous retrievals of aerosol absorption and vertical distribution over bright land surfaces are quite uncertain. We test a merger of RSP and High Spectral Resolution Lidar (HSRL) data with observations of boreal forest fire smoke, collected during the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS). During ARCTAS, the RSP and HSRL instruments were mounted on the same aircraft, and validation data were provided by instruments on an aircraft flying a coordinated flight pattern. We found that the lidar data did indeed improve aerosol retrievals using an optimal estimation method, although not primarily because of the constraints imposed on the aerosol vertical distribution. The more useful piece of information from the HSRL was the total column aerosol optical depth, which was used to select the initial value (optimization starting point) of the aerosol number concentration. When ground based sun photometer network climatologies of number concentration were used as an initial value, we found that roughly half of the retrievals had unrealistic sizes and imaginary indices, even though the retrieved spectral optical depths agreed within uncertainties to

  17. Spatio-temporal precipitation climatology over complex terrain using a censored additive regression model.

    PubMed

    Stauffer, Reto; Mayr, Georg J; Messner, Jakob W; Umlauf, Nikolaus; Zeileis, Achim

    2017-06-15

    Flexible spatio-temporal models are widely used to create reliable and accurate estimates for precipitation climatologies. Most models are based on square root transformed monthly or annual means, where a normal distribution seems to be appropriate. This assumption becomes invalid on a daily time scale as the observations involve large fractions of zero observations and are limited to non-negative values. We develop a novel spatio-temporal model to estimate the full climatological distribution of precipitation on a daily time scale over complex terrain using a left-censored normal distribution. The results demonstrate that the new method is able to account for the non-normal distribution and the large fraction of zero observations. The new climatology provides the full climatological distribution on a very high spatial and temporal resolution, and is competitive with, or even outperforms existing methods, even for arbitrary locations.

  18. Combustion Aerosol over Marine Stratus: Long Range Transport, Subsidence and Aerosol-Cloud Interactions over the South East Pacific

    NASA Astrophysics Data System (ADS)

    Clarke, A. D.; Snider, J.; Freitag, S.; Feingold, G.; Campos, T. L.; Breckhovskikh, V.; Kazil, J.

    2011-12-01

    The worlds largest stratus deck over the South East Pacific (SEP) was a study target for the VOCALS (http://www.eol.ucar.edu/projects/vocals/) experiment in October 2008. Aerosol-cloud interactions were one major goal of several ship and aircraft studies including results from 14 flights of the NCAR C-130 aircraft reported here. Each flight covered about a 1000 km range with multiple profiles and legs below, in and above the Sc deck. Strong aerosol sources along the coast of Chile were expected and found to influence cloud condensation nuclei (CCN) in coastal clouds. However; "rivers" of elevated CO, black carbon (BC) associated with combustion aerosol effective as CCN at <0.3%S were also common in subsiding FT air overlying the extensive Sc deck for over 1000km offshore. This subsidence, linked to the Hadley circulation, brought in aerosol from sources over the western Pacific as well as South America. Observed entrainment of this aerosol appeared linked to cloud related turbulence. When present, this combustion aerosol increased available CCN and decreased effective radius compared to clouds in "clean" MBL air advected from the South Pacific. We hypothesize that this entrainment can help buffer MBL clouds over the SEP against depletion of CCN by drizzle. This may delay transition of closed cell to open cell convection, potentially leading to increased lifetimes of Sc clouds that entrain such aerosol.

  19. Characterizing the Vertical Distribution of Aerosols Over the ARM SGP Site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Richard Ferrare, Connor Flynn, David Turner

    This project focused on: 1) evaluating the performance of the DOE ARM SGP Raman lidar system in measuring profiles of water vapor and aerosols, and 2) the use of the Raman lidar measurements of aerosol and water vapor profiles for assessing the vertical distribution of aerosols and water vapor simulated by global transport models and examining diurnal variability of aerosols and water vapor. The highest aerosol extinction was generally observed close to the surface during the nighttime just prior to sunrise. The high values of aerosol extinction are most likely associated with increased scattering by hygroscopic aerosols, since the correspondingmore » average relative humidity values were above 70%. After sunrise, relative humidity and aerosol extinction below 500 m decreased with the growth in the daytime convective boundary layer. The largest aerosol extinction for altitudes above 1 km occurred during the early afternoon most likely as a result of the increase in relative humidity. The water vapor mixing ratio profiles generally showed smaller variations with altitude between day and night. We also compared simultaneous measurements of relative humidity, aerosol extinction, and aerosol optical thickness derived from the ARM SGP Raman lidar and in situ instruments on board a small aircraft flown routinely over the ARM SGP site. In contrast, the differences between the CARL and IAP aerosol extinction measurements are considerably larger. Aerosol extinction derived from the IAP measurements is, on average, about 30-40% less than values derived from the Raman lidar. The reasons for this difference are not clear, but may be related to the corrections for supermicron scattering and relative humidity that were applied to the IAP data. The investigators on this project helped to set up a major field mission (2003 Aerosol IOP) over the DOE ARM SGP site. One of the goals of the mission was to further evaluate the aerosol and water vapor retrievals from this lidar system

  20. Modeling the Absorbing Aerosol Index

    NASA Technical Reports Server (NTRS)

    Penner, Joyce; Zhang, Sophia

    2003-01-01

    We propose a scheme to model the absorbing aerosol index and improve the biomass carbon inventories by optimizing the difference between TOMS aerosol index (AI) and modeled AI with an inverse model. Two absorbing aerosol types are considered, including biomass carbon and mineral dust. A priori biomass carbon source was generated by Liousse et al [1996]. Mineral dust emission is parameterized according to surface wind and soil moisture using the method developed by Ginoux [2000]. In this initial study, the coupled CCM1 and GRANTOUR model was used to determine the aerosol spatial and temporal distribution. With modeled aerosol concentrations and optical properties, we calculate the radiance at the top of the atmosphere at 340 nm and 380 nm with a radiative transfer model. The contrast of radiance at these two wavelengths will be used to calculate AI. Then we compare the modeled AI with TOMS AI. This paper reports our initial modeling for AI and its comparison with TOMS Nimbus 7 AI. For our follow-on project we will model the global AI with aerosol spatial and temporal distribution recomputed from the IMPACT model and DAO GEOS-1 meteorology fields. Then we will build an inverse model, which applies a Bayesian inverse technique to optimize the agreement of between model and observational data. The inverse model will tune the biomass burning source strength to reduce the difference between modelled AI and TOMS AI. Further simulations with a posteriori biomass carbon sources from the inverse model will be carried out. Results will be compared to available observations such as surface concentration and aerosol optical depth.

  1. Laboratory Experiments and Instrument Intercomparison Studies of Carbonaceous Aerosol Particles

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Davidovits, Paul

    Aerosols containing black carbon (and some specific types of organic particulate matter) directly absorb incoming light, heating the atmosphere. In addition, all aerosol particles backscatter solar light, leading to a net-cooling effect. Indirect effects involve hydrophilic aerosols, which serve as cloud condensation nuclei (CCN) that affect cloud cover and cloud stability, impacting both atmospheric radiation balance and precipitation patterns. At night, all clouds produce local warming, but overall clouds exert a net-cooling effect on the Earth. The effect of aerosol radiative forcing on climate may be as large as that of the greenhouse gases, but predominantly opposite in sign andmore » much more uncertain. The uncertainties in the representation of aerosol interactions in climate models makes it problematic to use model projections to guide energy policy. The objective of our program is to reduce the uncertainties in the aerosol radiative forcing in the two areas highlighted in the ASR Science and Program Plan. That is, (1) addressing the direct effect by correlating particle chemistry and morphology with particle optical properties (i.e. absorption, scattering, extinction), and (2) addressing the indirect effect by correlating particle hygroscopicity and CCN activity with particle size, chemistry, and morphology. In this connection we are systematically studying particle formation, oxidation, and the effects of particle coating. The work is specifically focused on carbonaceous particles where the uncertainties in the climate relevant properties are the highest. The ongoing work consists of laboratory experiments and related instrument inter-comparison studies both coordinated with field and modeling studies, with the aim of providing reliable data to represent aerosol processes in climate models. The work is performed in the aerosol laboratory at Boston College. At the center of our laboratory setup are two main sources for the production of aerosol

  2. Time-series MODIS satellite and in-situ data for spatio-temporal distribution of aerosol pollution assessment over Bucharest metropolitan area

    NASA Astrophysics Data System (ADS)

    Zoran, Maria A.; Savastru, Roxana S.; Savastru, Dan M.

    2015-10-01

    With the increasing industrialization and urbanization, especially in the metropolis regions, aerosol pollution has highly negative effects on environment. Urbanization is responsible of three major changes that may have impact on the urban atmosphere: replacement of the natural surfaces with buildings and impermeable pavements, heat of anthropogenic origin and air pollution. The importance of aerosols for radiative and atmospheric chemical processes is widely recognized. They can scatter and/or absorb solar radiation leading to changes of the radiation budget. Also, the so-called indirect effect of aerosols describes the cloud-aerosol interactions, which can modify the chemical and physical processes in the atmosphere. Their high spatial variability and short lifetime make spaceborne sensors especially well suited for their observation. Remote sensing is a key application in global-change science and urban climatology. Since the launch of the MODerate resolution Imaging Spectroradiometer (MODIS) there is detailed global aerosol information available, both over land and oceans The aerosol parameters can be measured directly in situ or derived from satellite remote sensing observations. All these methods are important and complementary. The objective of this work was to document the seasonal and inter-annual patterns of the aerosol pollution particulate matter in two size fractions (PM10 and PM2.5) loading and air quality index (AQI) over Bucharest metropolitan area in Romania based on in-situ and MODIS (Terra-Moderate Resolution Imaging Spectoradiometer) satellite time series data over 2010-2012 period. Accurate information of urban air pollution is required for environmental and health policy, but also to act as a basis for designing and stratifying future monitoring networks.

  3. Aqueous aerosol SOA formation: impact on aerosol physical properties.

    PubMed

    Woo, Joseph L; Kim, Derek D; Schwier, Allison N; Li, Ruizhi; McNeill, V Faye

    2013-01-01

    Organic chemistry in aerosol water has recently been recognized as a potentially important source of secondary organic aerosol (SOA) material. This SOA material may be surface-active, therefore potentially affecting aerosol heterogeneous activity, ice nucleation, and CCN activity. Aqueous aerosol chemistry has also been shown to be a potential source of light-absorbing products ("brown carbon"). We present results on the formation of secondary organic aerosol material in aerosol water and the associated changes in aerosol physical properties from GAMMA (Gas-Aerosol Model for Mechanism Analysis), a photochemical box model with coupled gas and detailed aqueous aerosol chemistry. The detailed aerosol composition output from GAMMA was coupled with two recently developed modules for predicting a) aerosol surface tension and b) the UV-Vis absorption spectrum of the aerosol, based on our previous laboratory observations. The simulation results suggest that the formation of oligomers and organic acids in bulk aerosol water is unlikely to perturb aerosol surface tension significantly. Isoprene-derived organosulfates are formed in high concentrations in acidic aerosols under low-NO(x) conditions, but more experimental data are needed before the potential impact of these species on aerosol surface tension may be evaluated. Adsorption of surfactants from the gas phase may further suppress aerosol surface tension. Light absorption by aqueous aerosol SOA material is driven by dark glyoxal chemistry and is highest under high-NO(x) conditions, at high relative humidity, in the early morning hours. The wavelength dependence of the predicted absorption spectra is comparable to field observations and the predicted mass absorption efficiencies suggest that aqueous aerosol chemistry can be a significant source of aerosol brown carbon under urban conditions.

  4. An overview of regional and local characteristics of aerosols in South Africa using satellite, ground, and modeling data

    PubMed Central

    Hersey, S. P.; Garland, R. M.; Crosbie, E.; Shingler, T.; Sorooshian, A.; Piketh, S.; Burger, R.

    2015-01-01

    We present a comprehensive overview of particulate air quality across the five major metropolitan areas of South Africa (Cape Town, Bloemfontein, Johannesburg and Tshwane (Gauteng Province), the Industrial Highveld Air Quality Priority Area (HVAPA), and Durban), based on a decadal (1 January 2000 to 31 December 2009) aerosol climatology from multiple satellite platforms and detailed analysis of ground-based data from 19 sites throughout Gauteng Province. Satellite analysis was based on aerosol optical depth (AOD) from MODIS Aqua and Terra (550 nm) and MISR (555 nm) platforms, Ångström Exponent (α) from MODIS Aqua (550/865 nm) and Terra (470/660 nm), ultraviolet aerosol index (UVAI) from TOMS, and results from the Goddard Ozone Chemistry Aerosol Radiation and Transport (GOCART) model. At continentally influenced sites, AOD, α, and UVAI reach maxima (0.12–0.20, 1.0–1.8, and 1.0–1.2, respectively) during austral spring (September–October), coinciding with a period of enhanced dust generation and the maximum integrated intensity of close-proximity and subtropical fires identified by MODIS Fire Information for Resource Management System (FIRMS). Minima in AOD, α, and UVAI occur during winter. Results from ground monitoring indicate that low-income township sites experience by far the worst particulate air quality in South Africa, with seasonally averaged PM10 concentrations as much as 136 % higher in townships that in industrial areas. We report poor agreement between satellite and ground aerosol measurements, with maximum surface aerosol concentrations coinciding with minima in AOD, α, and UVAI. This result suggests that remotely sensed data are not an appropriate surrogate for ground air quality in metropolitan South Africa. PMID:26312061

  5. Aerosol algorithm evaluation within aerosol-CCI

    NASA Astrophysics Data System (ADS)

    Kinne, Stefan; Schulz, Michael; Griesfeller, Jan

    Properties of aerosol retrievals from space are difficult. Even data from dedicated satellite sensors face contaminations which limit the accuracy of aerosol retrieval products. Issues are the identification of complete cloud-free scenes, the need to assume aerosol compositional features in an underdetermined solution space and the requirement to characterize the background at high accuracy. Usually the development of aerosol is a slow process, requiring continuous feedback from evaluations. To demonstrate maturity, these evaluations need to cover different regions and seasons and many different aerosol properties, because aerosol composition is quite diverse and highly variable in space and time, as atmospheric aerosol lifetimes are only a few days. Three years ago the ESA Climate Change Initiative started to support aerosol retrieval efforts in order to develop aerosol retrieval products for the climate community from underutilized ESA satellite sensors. The initial focus was on retrievals of AOD (a measure for the atmospheric column amount) and of Angstrom (a proxy for aerosol size) from the ATSR and MERIS sensors on ENVISAT. The goal was to offer retrieval products that are comparable or better in accuracy than commonly used NASA products of MODIS or MISR. Fortunately, accurate reference data of ground based sun-/sky-photometry networks exist. Thus, retrieval assessments could and were conducted independently by different evaluation groups. Here, results of these evaluations for the year 2008 are summarized. The capability of these newly developed retrievals is analyzed and quantified in scores. These scores allowed a ranking of competing efforts and also allow skill comparisons of these new retrievals against existing and commonly used retrievals.

  6. Application of the CALIOP Layer Product to Evaluate the Vertical Distribution of Aerosols Estimated by Global Models: AeroCom Phase I Results

    NASA Technical Reports Server (NTRS)

    Koffi, Brigitte; Schulz, Michael; Breon, Francois-Marie; Griesfeller, Jan; Winker, David; Balkanski, Yves; Bauer, Susanne; Berntsen, Terje; Chin, Mian; Collins, William D.; hide

    2012-01-01

    The CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) layer product is used for a multimodel evaluation of the vertical distribution of aerosols. Annual and seasonal aerosol extinction profiles are analyzed over 13 sub-continental regions representative of industrial, dust, and biomass burning pollution, from CALIOP 2007-2009 observations and from AeroCom (Aerosol Comparisons between Observations and Models) 2000 simulations. An extinction mean height diagnostic (Z-alpha) is defined to quantitatively assess the models' performance. It is calculated over the 0-6 km and 0-10 km altitude ranges by weighting the altitude of each 100 m altitude layer by its aerosol extinction coefficient. The mean extinction profiles derived from CALIOP layer products provide consistent regional and seasonal specificities and a low inter-annual variability. While the outputs from most models are significantly correlated with the observed Z-alpha climatologies, some do better than others, and 2 of the 12 models perform particularly well in all seasons. Over industrial and maritime regions, most models show higher Z-alpha than observed by CALIOP, whereas over the African and Chinese dust source regions, Z-alpha is underestimated during Northern Hemisphere Spring and Summer. The positive model bias in Z-alpha is mainly due to an overestimate of the extinction above 6 km. Potential CALIOP and model limitations, and methodological factors that might contribute to the differences are discussed.

  7. Characterization of aerosols produced by surgical procedures

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yeh, H.C.; Muggenburg, B.A.; Lundgren, D.L.

    1994-07-01

    In many surgeries, especially orthopedic procedures, power tools such as saws and drills are used. These tools may produce aerosolized blood and other biological material from bone and soft tissues. Surgical lasers and electrocautery tools can also produce aerosols when tissues are vaporized and condensed. Studies have been reported in the literature concerning production of aerosols during surgery, and some of these aerosols may contain infectious material. Garden et al. (1988) reported the presence of papilloma virus DNA in the fumes produced from laser surgery, but the infectivity of the aerosol was not assessed. Moon and Nininger (1989) measured themore » size distribution and production rate of emissions from laser surgery and found that particles were generally less than 0.5 {mu}m diameter. More recently there has been concern expressed over the production of aerosolized blood during surgical procedures that require power tools. In an in vitro study, the production of an aerosol containing the human immunodeficiency virus (HIV) was reported when power tools were used to cut tissues with blood infected with HIV. Another study measured the size distribution of blood aerosols produced by surgical power tools and found blood-containing particles in a number of size ranges. Health care workers are anxious and concerned about whether surgically produced aerosols are inspirable and can contain viable pathogens such as HIV. Other pathogens such as hepatitis B virus (HBV) are also of concern. The Occupational Safety and Health funded a project at the National Institute for Inhalation Toxicology Research Institute to assess the extent of aerosolization of blood and other tissues during surgical procedures. This document reports details of the experimental and sampling approach, methods, analyses, and results on potential production of blood-associated aerosols from surgical procedures in the laboratory and in the hospital surgical suite.« less

  8. The surface climatology of the Ross Ice Shelf Antarctica.

    PubMed

    Costanza, Carol A; Lazzara, Matthew A; Keller, Linda M; Cassano, John J

    2016-12-01

    The University of Wisconsin-Madison Antarctic Automatic Weather Station (AWS) project has been making meteorological surface observations on the Ross Ice Shelf (RIS) for approximately 30 years. This network offers the most continuous set of routine measurements of surface meteorological variables in this region. The Ross Island area is excluded from this study. The surface climate of the RIS is described using the AWS measurements. Temperature, pressure, and wind data are analysed on daily, monthly, seasonal, and annual time periods for 13 AWS across the RIS. The AWS are separated into three representative regions - central, coastal, and the area along the Transantarctic Mountains - in order to describe specific characteristics of sections of the RIS. The climatology describes general characteristics of the region and significant changes over time. The central AWS experiences the coldest mean temperature, and the lowest resultant wind speed. These AWSs also experience the coldest potential temperatures with a minimum of 209.3 K at Gill AWS. The AWS along the Transantarctic Mountains experiences the warmest mean temperature, the highest mean sea-level pressure, and the highest mean resultant wind speed. Finally, the coastal AWS experiences the lowest mean pressure. Climate indices (MEI, SAM, and SAO) are compared to temperature and pressure data of four of the AWS with the longest observation periods, and significant correlation is found for most AWS in sea-level pressure and temperature. This climatology study highlights characteristics that influence the climate of the RIS, and the challenges of maintaining a long-term Antarctic AWS network. Results from this effort are essential for the broader Antarctic meteorology community for future research.

  9. The surface climatology of the Ross Ice Shelf Antarctica

    PubMed Central

    Lazzara, Matthew A.; Keller, Linda M.; Cassano, John J.

    2016-01-01

    ABSTRACT The University of Wisconsin‐Madison Antarctic Automatic Weather Station (AWS) project has been making meteorological surface observations on the Ross Ice Shelf (RIS) for approximately 30 years. This network offers the most continuous set of routine measurements of surface meteorological variables in this region. The Ross Island area is excluded from this study. The surface climate of the RIS is described using the AWS measurements. Temperature, pressure, and wind data are analysed on daily, monthly, seasonal, and annual time periods for 13 AWS across the RIS. The AWS are separated into three representative regions – central, coastal, and the area along the Transantarctic Mountains – in order to describe specific characteristics of sections of the RIS. The climatology describes general characteristics of the region and significant changes over time. The central AWS experiences the coldest mean temperature, and the lowest resultant wind speed. These AWSs also experience the coldest potential temperatures with a minimum of 209.3 K at Gill AWS. The AWS along the Transantarctic Mountains experiences the warmest mean temperature, the highest mean sea‐level pressure, and the highest mean resultant wind speed. Finally, the coastal AWS experiences the lowest mean pressure. Climate indices (MEI, SAM, and SAO) are compared to temperature and pressure data of four of the AWS with the longest observation periods, and significant correlation is found for most AWS in sea‐level pressure and temperature. This climatology study highlights characteristics that influence the climate of the RIS, and the challenges of maintaining a long‐term Antarctic AWS network. Results from this effort are essential for the broader Antarctic meteorology community for future research. PMID:28008213

  10. Monthly mean global climatology of temperature, wind, geopotential height, and pressure for 0 - 120 km

    NASA Technical Reports Server (NTRS)

    Fleming, Eric L.; Chandra, Sushil; Schoeberl, Mark R.; Barnett, John J.

    1988-01-01

    A monthly mean climatology is presented of temperature, wind, and geopotential height with nearly pole-to-pole coverage (80 S to 80 N) for 0 to 210 km, which can be used as a function of altitude and pressure. The purpose is to provide a reference for various atmospheric research and analysis activities. Data sources and methods of computation are described; in general, hydrostatic and thermal wind balance are maintained at all levels and latitudes. As observed in a series of cross-sectional plots, this climatology accurately reproduces most of the characteristic features of the atmosphere such as equatorial wind and the general structure of the tropopause, stratopause, and mesopause. A series of zonal wind profiles is also represented comparing this climatological wind with monthly mean climatological direct wind measurements in the upper mesosphere and lower thermosphere. The temperature and zonal wind climatology at stratospheric levels is compared with corresponding data from the National Meteorological Center, and general agreement is observed between the two data sets. Tables of the climatological values as a function of latitude and height for each month are contained in Appendix B, and are also available in floppy disk.

  11. Novel Co:MgF2 lidar for aerosol profiler

    NASA Technical Reports Server (NTRS)

    Acharekar, M. A.

    1993-01-01

    Lidars are of great interest because of their unique capabilities in remote sensing applications in sounding of the atmosphere, meteorology, and climatology. In this small business innovative research (SBIR) phase II program, laser sources including Co:MgF2, CTH:YAG, CTH:YSGG, CT:YAG, and Er:Glass were evaluated. Modulator of fused silica and TeO2 materials with Brewster's angle end faces were used with these lasers as acousto-optical (AO) Q-switches. A higher hold-off energy and hence a higher Q-switched energy was obtained by using a high power RF driver. The report provides performance characteristics of these lasers. The tunable (1.75-2.50 microns) Co:MgF2 laser damaged the TeO2 Q-switch cell. However, the CTH:YAG laser operating at 2.09 microns provided output energy of over 300 mJ/p in 50 ns pulse width using the fused silica Q-switch. This Q-switched CTH:YAG laser was used in a breadboard vertical aerosol profiler. A 40 cm diameter telescope, InSb and InGaAs detectors were used in the receiver. The data obtained using this lidar is provided in the report. The data shows that the eye safe lidar using CTH:YAG laser for the vertical aerosol density and range measurements is the viable approach.

  12. Contributions of changes in climatology and perturbation and the resulting nonlinearity to regional climate change.

    PubMed

    Adachi, Sachiho A; Nishizawa, Seiya; Yoshida, Ryuji; Yamaura, Tsuyoshi; Ando, Kazuto; Yashiro, Hisashi; Kajikawa, Yoshiyuki; Tomita, Hirofumi

    2017-12-20

    Future changes in large-scale climatology and perturbation may have different impacts on regional climate change. It is important to understand the impacts of climatology and perturbation in terms of both thermodynamic and dynamic changes. Although many studies have investigated the influence of climatology changes on regional climate, the significance of perturbation changes is still debated. The nonlinear effect of these two changes is also unknown. We propose a systematic procedure that extracts the influences of three factors: changes in climatology, changes in perturbation and the resulting nonlinear effect. We then demonstrate the usefulness of the procedure, applying it to future changes in precipitation. All three factors have the same degree of influence, especially for extreme rainfall events. Thus, regional climate assessments should consider not only the climatology change but also the perturbation change and their nonlinearity. This procedure can advance interpretations of future regional climates.

  13. Anthropogenic aerosols and the distribution of past large-scale precipitation change

    DOE PAGES

    Wang, Chien

    2015-12-28

    In this paper, the climate response of precipitation to the effects of anthropogenic aerosols is a critical while not yet fully understood aspect in climate science. Results of selected models that participated the Coupled Model Intercomparison Project Phase 5 and the data from the Twentieth Century Reanalysis Project suggest that, throughout the tropics and also in the extratropical Northern Hemisphere, aerosols have largely dominated the distribution of precipitation changes in reference to the preindustrial era in the second half of the last century. Aerosol-induced cooling has offset some of the warming caused by the greenhouse gases from the tropics tomore » the Arctic and thus formed the gradients of surface temperature anomaly that enable the revealed precipitation change patterns to occur. Improved representation of aerosol-cloud interaction has been demonstrated as the key factor for models to reproduce consistent distributions of past precipitation change with the reanalysis data.« less

  14. Aerosol optical properties and types over the tropical urban region of Hyderabad, India

    NASA Astrophysics Data System (ADS)

    Kharol, Shailesh Kumar; Kaskaoutis, D. G.; Rani Sharma, Anu; Kvs, Badarinath; Kambezidis, H. D.

    outbreaks), while the presence of mixed aerosols, without dominance of the coarse or accumulation mode is the usual situation. According to the analysis the three individual components of differing origin, composition and optical characteristics are, a) an urban/industrial aerosol type composed of aerosols produced locally and all year round by combustion activities in the city or long-range transported (mainly in spring) biomass burning, b) an aerosol type of mineral origin raised by the wind in the deserts (mainly in premonsoon) or constitutes coarse-mode aerosols under high relative humidity conditions mainly in the monsoon period, and c) an aerosol type with a marine influence under background conditions occurred in monsoon and postmonsoon periods. Nevertheless, the mixed or undetermined aerosol type dominates with percentages varying from 44.3% (premonsoon) to 72.9% (postmonsoon). Spec-tral AOD and α data are analyzed to obtain information about the adequacy of the simple use of the ˚ngstrüm exponent for characterizing the aerosols. This is achieved by taking advantage A of the spectral variation of lnAOD vs lnλ, the so-called curvature. The results show that the spectral curvature can be effectively used as a tool for aerosol types discrimination, since the fine-mode aerosols exhibit negative curvature, while the coarse-mode particles positive. The present study is among the first over Hyderabad focusing on the seasonal pattern of aerosol properties and types and aiming at associating them with local emissions, regional climatology and long-range transport. Keywords: AOD, aerosol types; sun photometer; back trajectories; Hyderabad; India

  15. Spectroscopic characterization of Antarctic marine aerosol

    NASA Astrophysics Data System (ADS)

    Paglione, Marco; Zanca, Nicola; Rinaldi, Matteo; Dall'osto, Manuel; Simo, Rafel; Facchini, Maria Cristina; Decesari, Stefano

    2017-04-01

    Marine aerosol constitutes an important and not thoroughly investigated natural aerosol system. In particular, the poor knowledge of the physical-chemical properties of primary (sea-spray) and secondary particles, especially over biologically active seawaters, affects the current capability of modeling the effect of marine aerosol on climate (O'Dowd et al., 2004). In polar regions, surface seawater composition and its exchanges with the atmosphere is complicated also by the presence of sea-ice and of the variety of micro-organisms (viruses, prokaryotes and microalgae) living within it (Levasseur,2013). In the framework of the Spanish project PEGASO (Plankton-derived Emission of Gases and Aerosols in the Southern Ocean) submicron aerosol samples were collected during a 6 weeks long oceanographic cruise (2nd January 2015 - 11th February 2015) conducted in the regions of Antarctic Peninsula, South Orkney and South Georgia Islands, an area of the Southern Ocean characterized every summer by both large patches of productive waters (phytoplankton blooms) and sea-ice cover. The collected samples were analyzed by means of proton-Nuclear Magnetic Resonance (H-NMR) spectroscopy with aim of organic compounds characterization in terms of functional groups and specific molecular tracers identification (Decesari et al., 2011). H-NMR spectral features resulted quite variable among the different samples both in terms of relative abundance of main functional groups and in terms of presence of specific compounds. In all the samples were found biogenic markers, like low-molecular-weight alkyl-amines and methanesulphonate (MSA), of secondary origin (formed by the condensation of vapors onto particles). Resonance signals of other aliphatic compounds of possible primary origin, like lipids, aminoacids (e.g. alanine) and sugars (e.g. sucrose) are present in variable concentrations in the samples. A hierarchical cluster analysis applied on the NMR spectra allowed to identify similarities

  16. Experimental investigation of aerosol composition and growth rates

    NASA Astrophysics Data System (ADS)

    Wimmer, Daniela; Winkler, Paul; Kulmala, Markku; Petäjä, Tuukka

    2017-04-01

    Atmospheric aerosol particles have relevant influence on human lives. Human health is affected, as by breathing in the aerosol particles, they deposit in the lungs causing various health problems. Also they interfere indirectly and directly with sunlight, which affects the climate on Earth. Primary aerosol particles originate for example from anthropogenic sources, such as Diesel cars or natural sources such as dessert dust. Secondary aerosol particles are formed via condensation of low volatile gas phase compounds. First, small clusters consisting of a few gas molecules only are formed, which can then grow to bigger aerosol particles. These then form seeds for cloud droplets. The chemical composition of the cloud particles determines whether the cloud absorbs or scatters sunlight more. Intensive experimental and theoretical work has been put into understanding the details of the initial processes leading to the natural formation of these secondary aerosol particles. According to modelling studies, aerosol particles formed via the nucleation process are responsible for about 50% of the global cloud condensation nuclei concentration. With currently used methods, the chemical composition of small molecular clusters (up to 2nm in diameter) can be resolved. Also standard methods to determine aerosol particle composition at sizes >10 nm are available. Within this project, the aerosol particle composition in the 2-4 nm size range will be investigated experimentally. The setup will consist of a combination of an electrical method that allows determine the electrical mobility of the particles which then can be converted to a diameter. By letting the charged particles travel through a changing electrical field, they travel at different speeds according to their mobility. That allows to particles with certain mobilities, which then can be converted to a diameter. After the size selection, the particles are counted by means of optical detection. Condensation particle counters

  17. Determining Cloud Thermodynamic Phase from Micropulse Lidar Network Data

    NASA Technical Reports Server (NTRS)

    Lewis, Jasper R.; Campbell, James; Lolli, Simone; Tan, Ivy; Welton, Ellsworth J.

    2017-01-01

    Determining cloud thermodynamic phase is a critical factor in studies of Earth's radiation budget. Here we use observations from the NASA Micro Pulse Lidar Network (MPLNET) and thermodynamic profiles from the Goddard Earth Observing System, version 5 (GEOS-5) to distinguish liquid water, mixed-phase, and ice water clouds. The MPLNET provides sparse global, autonomous, and continuous measurements of clouds and aerosols which have been used in a number of scientific investigations to date. The use of a standardized instrument and a common suite of data processing algorithms with thorough uncertainty characterization allows for straightforward comparisons between sites. Lidars with polarization capabilities have recently been incorporated into the MPLNET project which allows, for the first time, the ability to infer a cloud thermodynamic phase. This presentation will look specifically at the occurrence of ice and mixed phase clouds in the temperature region of -10 C to -40 C for different climatological regions and seasons. We compare MPLNET occurrences of mixed-phase clouds to an historical climatology based on observations from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) spacecraft.

  18. Determining cloud thermodynamic phase from Micropulse Lidar Network data

    NASA Astrophysics Data System (ADS)

    Lewis, J. R.; Campbell, J. R.; Lolli, S.; Tan, I.; Welton, E. J.

    2017-12-01

    Determining cloud thermodynamic phase is a critical factor in studies of Earth's radiation budget. Here we use observations from the NASA Micropulse Lidar Network (MPLNET) and thermodynamic profiles from the Goddard Earth Observing System, version 5 (GEOS-5) to distinguish liquid water, mixed-phase, and ice water clouds. The MPLNET provides sparse global, autonomous, and continuous measurements of clouds and aerosols which have been used in a number of scientific investigations to date. The use of a standardized instrument and a common suite of data processing algorithms with thorough uncertainty characterization allows for straightforward comparisons between sites. Lidars with polarization capabilities have recently been incorporated into the MPLNET project which allows, for the first time, the ability to infer a cloud thermodynamic phase. This presentation will look specifically at the occurrence of ice and mixed phase clouds in the temperature region of 0 °C to -40 °C for different climatological regions and seasons. We compare MPLNET occurrences of mixed-phase clouds to an historical climatology based on observations from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) instrument aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) spacecraft.

  19. Arabian Sea tropical cyclones intensified by emissions of black carbon and other aerosols.

    PubMed

    Evan, Amato T; Kossin, James P; Chung, Chul Eddy; Ramanathan, V

    2011-11-02

    Throughout the year, average sea surface temperatures in the Arabian Sea are warm enough to support the development of tropical cyclones, but the atmospheric monsoon circulation and associated strong vertical wind shear limits cyclone development and intensification, only permitting a pre-monsoon and post-monsoon period for cyclogenesis. Thus a recent increase in the intensity of tropical cyclones over the northern Indian Ocean is thought to be related to the weakening of the climatological vertical wind shear. At the same time, anthropogenic emissions of aerosols have increased sixfold since the 1930s, leading to a weakening of the southwesterly lower-level and easterly upper-level winds that define the monsoonal circulation over the Arabian Sea. In principle, this aerosol-driven circulation modification could affect tropical cyclone intensity over the Arabian Sea, but so far no such linkage has been shown. Here we report an increase in the intensity of pre-monsoon Arabian Sea tropical cyclones during the period 1979-2010, and show that this change in storm strength is a consequence of a simultaneous upward trend in anthropogenic black carbon and sulphate emissions. We use a combination of observational, reanalysis and model data to demonstrate that the anomalous circulation, which is radiatively forced by these anthropogenic aerosols, reduces the basin-wide vertical wind shear, creating an environment more favourable for tropical cyclone intensification. Because most Arabian Sea tropical cyclones make landfall, our results suggest an additional impact on human health from regional air pollution.

  20. Situational Lightning Climatologies for Central Florida: Phase IV

    NASA Technical Reports Server (NTRS)

    Bauman, William H., III

    2009-01-01

    The threat of lightning is a daily concern during the warm season in Florida. Research has revealed distinct spatial and temporal distributions of lightning occurrence that are strongly influenced by large-scale atmospheric flow regimes. Previously, the Applied Meteorology Unit (AMU) calculated the gridded lightning climatologies based on seven flow regimes over Florida for 1-, 3- and 6-hr intervals in 5-, 10-,20-, and 30-NM diameter range rings around the Shuttle Landing Facility (SLF) and eight other airfields in the National Weather Service in Melbourne (NWS MLB) county warning area (CWA). In this update to the work, the AMU recalculated the lightning climatologies for using individual lightning strike data to improve the accuracy of the climatologies. The AMU included all data regardless of flow regime as one of the stratifications, added monthly stratifications, added three years of data to the period of record and used modified flow regimes based work from the AMU's Objective Lightning Probability Forecast Tool, Phase II. The AMU made changes so the 5- and 10-NM radius range rings are consistent with the aviation forecast requirements at NWS MLB, while the 20- and 30-NM radius range rings at the SLF assist the Spaceflight Meteorology Group in making forecasts for weather Flight Rule violations during Shuttle landings. The AMU also updated the graphical user interface with the new data.

  1. Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: Model-Relevant Observations and the Beneficiary Modeling Efforts in the Realm of the EVS-2 Project ORACLES

    NASA Technical Reports Server (NTRS)

    Redemann, Jens

    2018-01-01

    Globally, aerosols remain a major contributor to uncertainties in assessments of anthropogenically-induced changes to the Earth climate system, despite concerted efforts using satellite and suborbital observations and increasingly sophisticated models. The quantification of direct and indirect aerosol radiative effects, as well as cloud adjustments thereto, even at regional scales, continues to elude our capabilities. Some of our limitations are due to insufficient sampling and accuracy of the relevant observables, under an appropriate range of conditions to provide useful constraints for modeling efforts at various climate scales. In this talk, I will describe (1) the efforts of our group at NASA Ames to develop new airborne instrumentation to address some of the data insufficiencies mentioned above; (2) the efforts by the EVS-2 ORACLES project to address aerosol-cloud-climate interactions in the SE Atlantic and (3) time permitting, recent results from a synergistic use of A-Train aerosol data to test climate model simulations of present-day direct radiative effects in some of the AEROCOM phase II global climate models.

  2. Aerosol direct and indirect radiative effect over Eastern Mediterranean

    NASA Astrophysics Data System (ADS)

    Georgoulias, Aristeidis; Alexandri, Georgia; Zanis, Prodromos; Ntogras, Christos; Poeschl, Ulrich; Kourtidis, Kostas

    In this work, we present results from the QUADIEEMS project which is focused on the aerosol-cloud relations and the aerosol direct and indirect radiative effect over the region of Eastern Mediterranean. First, a gridded dataset at a resolution of 0.1x0.1 degrees (~10km) with aerosol and cloud related parameters was compiled, using level-2 satellite observations from MODIS TERRA (3/2000-12/2012) and AQUA (7/2002-12/2012). The aerosol gridded dataset has been validated against sunphotometric measurements from 12 AERONET ground stations, showing that generally MODIS overestimates aerosol optical depth (AOD550). Then, the AOD550 and fine mode ratio (FMR550) data from MODIS were combined with aerosol index (AI) data from the Earth Probe TOMS and OMI satellite sensors, wind field data from the ERA-interim reanalysis and AOD550 data for various aerosol types from the GOCART model and the MACC reanalysis to quantify the relative contribution of different aerosol types (marine, dust, anthropogenic, fine-mode natural) to the total AOD550. The aerosol-cloud relations over the region were investigated with the use of the joint high resolution aerosol-cloud gridded dataset. Specifically, we focused on the seasonal relations between the cloud droplet number concentration (CDNC) and AOD550. The aerosol direct and first indirect radiative effect was then calculated for each aerosol type separately making use of the aerosol relative contribution to the total AOD550, the CDND-AOD550 relations and satellite-based parameterizations. The direct radiative effect was also quantified using simulations from a regional climate model (REGCM4), simulations with a radiative transfer model (SBDART) and the three methods were finally intervalidated.

  3. Wind waves climatology of the Southeast Pacific Ocean

    NASA Astrophysics Data System (ADS)

    Aguirre, Catalina; Rutllant, José; Falvey, Mark

    2017-04-01

    The Southeast Pacific coast still lacks a high-resolution wave hindcast and a detailed description of its wave climatology. Since buoy wave measurements are particularly scarce along the coast of South America, a model hindcast forced with wind information derived from atmospheric Reanalysis seems an attractive way to generate a wave climatology in this poorly studied region, providing far better spatial and temporal coverage than can be achieved using observational data alone. Here, the climatology of wind waves over the Southeast Pacific is analyzed using a 32-year hindcast from the WaveWatch III model, complemented by satellite-derived Significant Wave Height (SWH) and buoy measurements for validation. Using partitioned spectral data, a regional climatology of wind sea and swell parameters was constructed. In general, the simulated SWH shows a good agreement with satellite and in-situ SWH measurements. The spatial pattern of SWH is clearly influenced by the meridional variation of mean surface wind speed, where the stronger winds over the Southern Ocean play a significant role generating higher waves at higher latitudes. Nevertheless, regional features are observed in the annual variability of SWH, which are associated with the existence of atmospheric coastal low-level jets off the coast of Peru and central Chile. In particular, the seasonal variation of these synoptic scale jets shows a direct relationship with the annual variability of SWH. Off the coast of Peru at 15°S the coastal low-level jet is strongest during austral winter, increasing the wind sea SWH. In contrast, off central Chile, there is an important increase of wind sea SWH during summer. The seasonal variation of the wind sea component leads to a contrasting seasonal variation of the total SWH at these locations: off Peru the coastal jet amplifies the annual variability of SWH, while off Central Chile the annual variability of SWH is suppressed by the presence of the coastal jet.

  4. Regional aerosol emissions and temperature response: Local and remote climate impacts of regional aerosol forcing

    NASA Astrophysics Data System (ADS)

    Lewinschal, Anna; Ekman, Annica; Hansson, Hans-Christen

    2017-04-01

    Emissions of anthropogenic aerosols vary substantially over the globe and the short atmospheric residence time of aerosols leads to a highly uneven radiative forcing distribution, both spatially and temporally. Regional aerosol radiative forcing can, nevertheless, exert a large influence on the temperature field away from the forcing region through changes in heat transport or the atmospheric or ocean circulation. Moreover, the global temperature response distribution to aerosol forcing may vary depending on the geographical location of the forcing. In other words, the climate sensitivity in one region can vary depending on the location of the forcing. The surface temperature distribution response to changes in sulphate aerosol forcing caused by sulphur dioxide (SO2) emission perturbations in four different regions is investigated using the Norwegian Earth System Model (NorESM). The four regions, Europe, North America, East and South Asia, are all regions with historically high aerosol emissions and are relevant from both an air-quality and climate policy perspective. All emission perturbations are defined relative to the year 2000 emissions provided for the Coupled Model Intercomparison Project phase 5. The global mean temperature change per unit SO2 emission change is similar for all four regions for similar magnitudes of emissions changes. However, the global temperature change per unit SO2 emission in simulations where regional SO2 emission were removed is substantially higher than that obtained in simulations where regional SO2 emissions were increased. Thus, the climate sensitivity to regional SO2 emissions perturbations depends on the magnitude of the emission perturbation in NorESM. On regional scale, on the other hand, the emission perturbations in different geographical locations lead to different regional temperature responses, both locally and in remote regions. The results from the model simulations are used to construct regional temperature potential

  5. Flow Regime Based Climatologies of Lightning Probabilities for Spaceports and Airports

    NASA Technical Reports Server (NTRS)

    Bauman, William H., III; Sharp, David; Spratt, Scott; Lafosse, Richard A.

    2008-01-01

    The objective of this work was to provide forecasters with a tool to indicate the warm season climatological probability of one or more lightning strikes within a circle at a site within a specified time interval. This paper described the AMU work conducted in developing flow regime based climatologies of lightning probabilities for the SLF and seven airports in the NWS MLB CWA in east-central Florida. The paper also described the GUI developed by the AMU that is used to display the data for the operational forecasters. There were challenges working with gridded lightning data as well as the code that accompanied the gridded data. The AMU modified the provided code to be able to produce the climatologies of lightning probabilities based on eight flow regimes for 5-, 10-, 20-, and 30-n mi circles centered on eight sites in 1-, 3-, and 6-hour increments.

  6. Fast Adjustments of the Asian Summer Monsoon to Anthropogenic Aerosols

    NASA Astrophysics Data System (ADS)

    Li, Xiaoqiong; Ting, Mingfang; Lee, Dong Eun

    2018-01-01

    Anthropogenic aerosols are a major factor contributing to human-induced climate change, particularly over the densely populated Asian monsoon region. Understanding the physical processes controlling the aerosol-induced changes in monsoon rainfall is essential for reducing the uncertainties in the future projections of the hydrological cycle. Here we use multiple coupled and atmospheric general circulation models to explore the physical mechanisms for the aerosol-driven monsoon changes on different time scales. We show that anthropogenic aerosols induce an overall reduction in monsoon rainfall and circulation, which can be largely explained by the fast adjustments over land north of 20∘N. This fast response occurs before changes in sea surface temperature (SST), largely driven by aerosol-cloud interactions. However, aerosol-induced SST feedbacks (slow response) cause substantial changes in the monsoon meridional circulation over the oceanic regions. Both the land-ocean asymmetry and meridional temperature gradient are key factors in determining the overall monsoon circulation response.

  7. The Impact of Biogenic and Anthropogenic Atmospheric Aerosol on Climate in Egypt

    NASA Astrophysics Data System (ADS)

    Ibrahim, A. I.; Zakey, A.; Steiner, A. L.; Shokr, M. E.; El-Raey, M.; Ahmed, Y.; Al-Hadidi, A.; Zakey, A.

    2014-12-01

    Aerosols are indicators of air quality as they reduce visibility and adversely affect public health. Aerosol optical depth (AOD) is a measure of the radiation extinction due to interaction of radiation with aerosol particles in the atmosphere. Using this optical measure of atmospheric aerosols we explore the seasonal and annual patterns of aerosols from both anthropogenic and biogenic sources over Egypt. Here, we use an integrated environment-climate-aerosol model in conjunction with inversion technique to identify the aerosol particle size distribution over different locations in Egypt. The online-integrated Environment-Climate-Aerosol model (EnvClimA), which is based on the International Center for Theoretical Physics Regional Climate Model (ICTP-RegCM), is used to study the emission of different aerosols and their impact on climate parameters for a long-term base line simulation run over Egypt and North Africa. The global emission inventory is downscaled and remapping them over Egypt using local factors such as population, traffic and industrial activities to identify the sources of anthropogenic and biogenic emission from local emission over Egypt. The results indicated that the dominant natural aerosols over Egypt are dust emissions that frequently occur during the transitional seasons (Spring and Autumn). From the local observation we identify the number of dust and sand storm occurrences over Egypt. The Multiangle Imaging SpectroRadiometer (MISR) is used to identify the optical characterizations of different types of aerosols over Egypt. Modeled aerosol optical depth and MISR observed (at 555 nm) are compared from March 2000 through November 2013. The results identify that the MISR AOD captures the maximum peaks of AOD in March/April that coincide with the Khamasin dust storms. However, peaks in May are either due to photochemical reactions or anthropogenic activities. Note: This presentation is for a Partnerships for Enhanced Engagement in Research (PEER

  8. Classifying aerosol type using in situ surface spectral aerosol optical properties

    NASA Astrophysics Data System (ADS)

    Schmeisser, Lauren; Andrews, Elisabeth; Ogren, John A.; Sheridan, Patrick; Jefferson, Anne; Sharma, Sangeeta; Kim, Jeong Eun; Sherman, James P.; Sorribas, Mar; Kalapov, Ivo; Arsov, Todor; Angelov, Christo; Mayol-Bracero, Olga L.; Labuschagne, Casper; Kim, Sang-Woo; Hoffer, András; Lin, Neng-Huei; Chia, Hao-Ping; Bergin, Michael; Sun, Junying; Liu, Peng; Wu, Hao

    2017-10-01

    Knowledge of aerosol size and composition is important for determining radiative forcing effects of aerosols, identifying aerosol sources and improving aerosol satellite retrieval algorithms. The ability to extrapolate aerosol size and composition, or type, from intensive aerosol optical properties can help expand the current knowledge of spatiotemporal variability in aerosol type globally, particularly where chemical composition measurements do not exist concurrently with optical property measurements. This study uses medians of the scattering Ångström exponent (SAE), absorption Ångström exponent (AAE) and single scattering albedo (SSA) from 24 stations within the NOAA/ESRL Federated Aerosol Monitoring Network to infer aerosol type using previously published aerosol classification schemes.Three methods are implemented to obtain a best estimate of dominant aerosol type at each station using aerosol optical properties. The first method plots station medians into an AAE vs. SAE plot space, so that a unique combination of intensive properties corresponds with an aerosol type. The second typing method expands on the first by introducing a multivariate cluster analysis, which aims to group stations with similar optical characteristics and thus similar dominant aerosol type. The third and final classification method pairs 3-day backward air mass trajectories with median aerosol optical properties to explore the relationship between trajectory origin (proxy for likely aerosol type) and aerosol intensive parameters, while allowing for multiple dominant aerosol types at each station.The three aerosol classification methods have some common, and thus robust, results. In general, estimating dominant aerosol type using optical properties is best suited for site locations with a stable and homogenous aerosol population, particularly continental polluted (carbonaceous aerosol), marine polluted (carbonaceous aerosol mixed with sea salt) and continental dust/biomass sites

  9. Multi-model analysis of precipitation-related climatological extremes for the Carpathian Region

    NASA Astrophysics Data System (ADS)

    Kis, Anna; Pongracz, Rita; Bartholy, Judit

    2015-04-01

    As a consequence of global climate change, both frequency and intensity of climatological and meteorological extremes are likely to change. These will certainly further induce various effects on hydrological extremes. Although more frequent hot weather in summer and overall warmer climatic conditions compared to the past decades are quite straightforward direct consequences of global warming, the effects on precipitation might be less clear because the higher spatial and temporal variabilities might hide robust changing signals. Nevertheless, precipitation is one of the most important meteorological variables since it considerably affects natural ecosystems and cultivated vegetation as well, as most of human activities. Extreme precipitation events - both excessive, intense rainfalls and severe droughts - may result in severe environmental, agricultural, and economical disasters. For instance, excessive precipitation may induce floods, flash-floods, landslides, traffic accidents. On the other hand, the lack of precipitation for extended period and coincidental intense heat wave often lead to severe drought events, which certainly affect agricultural production negatively, and hence, food safety might also be threatened. In order to avoid or at least reduce the effects of these precipitation-related hazards, national and local communities need to develop regional adaptation strategies, and then, act according to them. For this purpose, climatological projections are needed as a scientific basis. Coarse resolution results of global climate model (GCM) simulations must be downscaled to regional and local scales, hence better serving decision-makers' and end-users' needs. Dynamical downscaling technique applies regional climate model (RCM) to provide fine resolution climatological estimations for the future. Thus, in this study 11 completed RCM simulations with 25 km horizontal resolution are used from the ENSEMBLES database taking into account SRES A1B scenario for

  10. Subvisual-thin cirrus lidar dataset for satellite verification and climatological research

    NASA Technical Reports Server (NTRS)

    Sassen, Kenneth; Cho, Byung S.

    1992-01-01

    A polarization (0.694 microns wavelength) lidar dataset for subvisual and thin (bluish-colored) cirrus clouds is drawn from project FIRE (First ISCCP Regional Experiment) extended time observations. The clouds are characterized by their day-night visual appearance; base, top, and optical midcloud heights and temperatures; measured physical and estimated optical cloud thicknesses; integrated linear depolarization ratios; and derived k/2 eta ratios. A subset of the data supporting 30 NOAA polar-orbiting satellite overpasses is given in tabular form to provide investigators with the means to test cloud retrieval algorithms and establish the limits of cirrus detectability from satellite measurements under various conditions. Climatologically, subvisual-thin cirrus appear to be higher, colder, and more strongly depolarizing than previously reported multilatitude cirrus, although similar k/2 eta that decrease with height and temperature are found.

  11. Does temperature nudging overwhelm aerosol radiative effects in regional integrated climate models?

    NASA Astrophysics Data System (ADS)

    He, Jian; Glotfelty, Timothy; Yahya, Khairunnisa; Alapaty, Kiran; Yu, Shaocai

    2017-04-01

    Nudging (data assimilation) is used in many regional integrated meteorology-air quality models to reduce biases in simulated climatology. However, in such modeling systems, temperature changes due to nudging could compete with temperature changes induced by radiatively active and hygroscopic short-lived tracers leading to two interesting dilemmas: when nudging is continuously applied, what are the relative sizes of these two radiative forces at regional and local scales? How do these two forces present in the free atmosphere differ from those present at the surface? This work studies these two issues by converting temperature changes due to nudging into pseudo radiative effects (PRE) at the surface (PRE_sfc), in troposphere (PRE_atm), and at the top of atmosphere (PRE_toa), and comparing PRE with the reported aerosol radiative effects (ARE). Results show that the domain-averaged PRE_sfc is smaller than ARE_sfc estimated in previous studies and this work, but could be significantly larger than ARE_sfc at local scales. PRE_atm is also much smaller than ARE_atm. These results indicate that appropriate nudging methodology could be applied to the integrated models to study aerosol radiative effects at continental/regional scales, but it should be treated with caution for local scale applications.

  12. Precipitation Climatology on Titan-like Exomoons.

    PubMed

    Tokano, Tetsuya

    2015-06-01

    The availability of liquid water on the surface on Earth's continents in part relies on the precipitation of water. This implies that the habitability of exomoons has to consider not only the surface temperature and atmospheric pressure for the presence of liquid water, but also the global precipitation climatology. This study explores the sensitivity of the precipitation climatology of Titan-like exomoons to these moons' orbital configuration using a global climate model. The precipitation rate primarily depends on latitude and is sensitive to the planet's obliquity and the moon's rotation rate. On slowly rotating moons the precipitation shifts to higher latitudes as obliquity is increased, whereas on quickly rotating moons the latitudinal distribution does not strongly depend on obliquity. Stellar eclipse can cause a longitudinal variation in the mean surface temperature and surface pressure between the subplanetary and antiplanetary side if the planet's obliquity and the moon's orbital distance are small. In this particular condition the antiplanetary side generally receives more precipitation than the subplanetary side. However, precipitation on exomoons with dense atmospheres generally occurs at any longitude in contrast to tidally locked exoplanets.

  13. NASA GLDAS Evapotranspiration Data and Climatology

    NASA Technical Reports Server (NTRS)

    Rui, Hualan; Beaudoing, Hiroko Kato; Teng, William L.; Vollmer, Bruce; Rodell, Matthew

    2012-01-01

    Evapotranspiration (ET) is the water lost to the atmosphere by evaporation and transpiration. ET is a shared component in the energy and water budget, therefore, a critical variable for global energy and water cycle and climate change studies. However, direct ET measurements and data acquisition are difficult and expensive, especially at the global level. Therefore, modeling is one common alternative for estimating ET. With the goal to generate optimal fields of land surface states and fluxes, the Global Land Data Assimilation System (GLDAS) has been generating quality-controlled, spatially and temporally consistent, terrestrial hydrologic data, including ET and other variables that affect evaporation and transpiration, such as temperature, precipitation, humidity, wind, soil moisture, heat flux, and solar radiation. This poster presents the long-term ET climatology (mean and monthly), derived from the 61-year GLDAS-2 monthly 1.0 deg x 1.0 deg. NOAH model Experiment-1 data, and describes the basic characteristics of spatial and seasonal variations of the climatology. The time series of GLDAS-2 precipitation and radiation, and ET are also discussed to show the improvement of GLDAS-2 forcing data and model output over those from GLDAS-1.

  14. Remote Sensing of Spectral Aerosol Properties: A Classroom Experience

    NASA Technical Reports Server (NTRS)

    Levy, Robert C.; Pinker, Rachel T.

    2006-01-01

    Bridging the gap between current research and the classroom is a major challenge to today s instructor, especially in the sciences where progress happens quickly. NASA Goddard Space Flight Center and the University of Maryland teamed up in designing a graduate class project intended to provide a hands-on introduction to the physical basis for the retrieval of aerosol properties from state-of-the-art MODIS observations. Students learned to recognize spectral signatures of atmospheric aerosols and to perform spectral inversions. They became acquainted with the operational MODIS aerosol retrieval algorithm over oceans, and methods for its evaluation, including comparisons with groundbased AERONET sun-photometer data.

  15. Using Long-Term Satellite Observations to Identify Sensitive Regimes and Active Regions of Aerosol Indirect Effects for Liquid Clouds Over Global Oceans

    NASA Astrophysics Data System (ADS)

    Zhao, Xuepeng; Liu, Yangang; Yu, Fangquan; Heidinger, Andrew K.

    2018-01-01

    Long-term (1981-2011) satellite climate data records of clouds and aerosols are used to investigate the aerosol-cloud interaction of marine water cloud from a climatology perspective. Our focus is on identifying the regimes and regions where the aerosol indirect effects (AIEs) are evident in long-term averages over the global oceans through analyzing the correlation features between aerosol loading and the key cloud variables including cloud droplet effective radius (CDER), cloud optical depth (COD), cloud water path (CWP), cloud top height (CTH), and cloud top temperature (CTT). An aerosol optical thickness (AOT) range of 0.13 < AOT < 0.3 is identified as the sensitive regime of the conventional first AIE where CDER is more susceptible to AOT than the other cloud variables. The first AIE that manifests as the change of long-term averaged CDER appears only in limited oceanic regions. The signature of aerosol invigoration of water clouds as revealed by the increase of cloud cover fraction (CCF) and CTH with increasing AOT at the middle/high latitudes of both hemispheres is identified for a pristine atmosphere (AOT < 0.08). Aerosol invigoration signature is also revealed by the concurrent increase of CDER, COD, and CWP with increasing AOT for a polluted marine atmosphere (AOT > 0.3) in the tropical convergence zones. The regions where the second AIE is likely to manifest in the CCF change are limited to several oceanic areas with high CCF of the warm water clouds near the western coasts of continents. The second AIE signature as represented by the reduction of the precipitation efficiency with increasing AOT is more likely to be observed in the AOT regime of 0.08 < AOT < 0.4. The corresponding AIE active regions manifested themselves as the decline of the precipitation efficiency are mainly limited to the oceanic areas downwind of continental aerosols. The sensitive regime of the conventional AIE identified in this observational study is likely associated with the

  16. Radiative effects of biomass burning aerosols and cloudiness on seasonal carbon cycle in the Amazon region

    NASA Astrophysics Data System (ADS)

    Moreira, D. S.; Longo, K.; Freitas, S.; Mercado, L. M.; Miller, J. B.; Rosario, N. M. E. D.; Gatti, L.; Yamasoe, M. A.

    2017-12-01

    The Amazon region is characterized by high cloudiness, mainly due to convective clouds during most of the year due to the high humidity, and heat availability. However, during the Austral winter, the northward movement of the inter-tropical convergence zone (ITCZ) from its climatological position, significantly reducing cloudiness and precipitation, facilitating vegetation fires. Consequently, during these dry months, biomass burning aerosols contribute to relatively high values of aerosol optical depth (AOD) in Amazonia, typically exceeding 1.0 in the 550 nm wavelength. Both clouds and aerosols scatter solar radiation, reducing the direct irradiance and increasing the diffuse fraction that reaches the surface, decreasing near surface temperature and increasing photosynthetically active radiation (PAR) availability. This, in turn, affects energy and CO2 fluxes within the vegetation canopy. We applied an atmospheric model fully coupled to terrestrial carbon cycle model to assess the relative impact of biomass burning aerosols and clouds on CO2 fluxes in the Amazon region. Our results indicate that during most of the year, gross primary productivity (GPP) is high mainly due to high soil moisture and high values of the diffuse fraction of solar irradiation due to cloudiness. Therefore, heterotrophic and autotrophic respiration are both high, increasing the NEE values (i.e. reducing the net land sink). On the other hand, during the dry season, with a significant reduction of cloudiness, the biomass burning aerosol is mainly responsible for the increase in the diffuse fraction of solar irradiation and the GPP of the forest. However, the low soil moisture during the dry season, especially in the eastern Amazon, reduces heterotrophic and autotrophic respiration and thus compensates for reduced GPP compared to the wet season. Different reasons, an anthropogenic one (human induced fires during the dry season) and a natural one (cloudiness), lead to a somewhat stable value

  17. Development of an Extratropical Storm Wind, Wave, and Water Level Climatology for the Offshore Mid-Atlantic

    DTIC Science & Technology

    2015-08-01

    ER D C/ CH L TR -1 5- 11 Development of an Extratropical Storm Wind, Wave, and Water Level Climatology for the Offshore Mid-Atlantic...Development of an Extratropical Storm Wind, Wave, and Water Level Climatology for the Offshore Mid-Atlantic Michael F. Forte Field Research Facility...standards for offshore wind farm design and to establish a 100-year (yr) extratropical wind speed, wave height, and water level climatology for the

  18. Ground-based Network and Supersite Measurements for Studying Aerosol Properties and Aerosol-Cloud Interactions

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Holben, Brent N.

    2008-01-01

    From radiometric principles, it is expected that the retrieved properties of extensive aerosols and clouds from reflected/emitted measurements by satellite (and/or aircraft) should be consistent with those retrieved from transmitted/emitted radiance observed at the surface. Although space-borne remote sensing observations contain large spatial domain, they are often plagued by contamination of surface signatures. Thus, ground-based in-situ and remote-sensing measurements, where signals come directly from atmospheric constituents, the sun, and the Earth-atmosphere interactions, provide additional information content for comparisons that confirm quantitatively the usefulness of the integrated surface, aircraft, and satellite datasets. The development and deployment of AERONET (AErosol RObotic NETwork) sunphotometer network and SMART-COMMIT (Surface-sensing Measurements for Atmospheric Radiative Transfer - Chemical, Optical & Microphysical Measurements of In-situ Troposphere) mobile supersite are aimed for the optimal utilization of collocated ground-based observations as constraints to yield higher fidelity satellite retrievals and to determine any sampling bias due to target conditions. To characterize the regional natural and anthropogenic aerosols, AERONET is an internationally federated network of unique sunphotometry that contains more than 250 permanent sites worldwide. Since 1993, there are more than 480 million aerosol optical depth observations and about 15 sites have continuous records longer than 10 years for annual/seasonal trend analyses. To quantify the energetics of the surface-atmosphere system and the atmospheric processes, SMART-COMMIT instrument into three categories: flux radiometer, radiance sensor and in-situ probe. Through participation in many satellite remote-sensing/retrieval and validation projects over eight years, SMART-COMMIT have gradually refine( and been proven vital for field deployment. In this paper, we will demonstrate the

  19. Aerosol contribution to the rapid warming of near-term climate under RCP 2.6

    NASA Astrophysics Data System (ADS)

    Chalmers, N.; Highwood, E. J.; Hawkins, E.; Sutton, R.; Wilcox, L. J.

    2012-09-01

    The importance of aerosol emissions for near term climate projections is investigated by analysing simulations with the HadGEM2-ES model under two different emissions scenarios: RCP2.6 and RCP4.5. It is shown that the near term warming projected under RCP2.6 is greater than under RCP4.5, even though the greenhouse gas forcing is lower. Rapid and substantial reductions in sulphate aerosol emissions due to a reduction of coal burning in RCP2.6 lead to a reduction in the negative shortwave forcing due to aerosol direct and indirect effects. Indirect effects play an important role over the northern hemisphere oceans, especially the subtropical northeastern Pacific where an anomaly of 5-10 Wm-2 develops. The pattern of surface temperature change is consistent with the expected response to this surface radiation anomaly, whilst also exhibiting features that reflect redistribution of energy, and feedbacks, within the climate system. These results demonstrate the importance of aerosol emissions as a key source of uncertainty in near term projections of global and regional climate.

  20. Comparisons of Airborne HSRL and Modeled Aerosol Profiles

    NASA Astrophysics Data System (ADS)

    Ferrare, R. A.; Burton, S. P.; Hostetler, C. A.; Hair, J. W.; Ismail, S.; Rogers, R. R.; Notari, A.; Berkoff, T.; Butler, C. F.; Collins, J. E., Jr.; Fenn, M. A.; Scarino, A. J.; Clayton, M.; Mueller, D.; Chemyakin, E.; Fast, J. D.; Berg, L. K.; Randles, C. A.; Colarco, P. R.; daSilva, A.

    2014-12-01

    Aerosol profiles derived from a regional and a global model are compared with aerosol profiles acquired by NASA Langley Research Center (LaRC) airborne High Spectral Resolution Lidars (HSRLs) during recent field missions. We compare simulated aerosol profiles obtained from the WRF-Chem regional model with those measured by the airborne HSRL-2 instrument over the Atlantic Ocean east of Cape Cod in July 2012 during the Department of Energy Two-Column Aerosol Project (TCAP). While deployed on the LaRC King Air during TCAP, HSRL-2 acquired profiles of aerosol extinction at 355 and 532 nm, as well as aerosol backscatter and depolarization at 355, 532, and 1064 nm. Additional HSRL-2 data products include profiles of aerosol type, mixed layer depth, and aerosol microphysical parameters (e.g. effective radius, concentration). The HSRL-2 and WRF-Chem aerosol profiles are compared along the aircraft flight tracks. HSRL-2 profiles acquired during the NASA Deriving Information on Surface Conditions from COlumn and VERtically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) mission over Houston during September 2013 are compared with the NASA Goddard Earth Observing System global model, version 5 (GEOS-5) profiles. In addition to comparing backscatter and extinction profiles, the fraction of aerosol extinction and optical thickness from various aerosol species from GEOS-5 are compared with aerosol extinction and optical thickness contributed by aerosol types derived from HSRL-2 data. We also compare aerosol profiles modeled by GEOS-5 with those measured by the airborne LaRC DIAL/HSRL instrument during August and September 2013 when it was deployed on the NASA DC-8 for the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) mission. DIAL/HSRL measured extinction (532 nm), backscatter (532 and 1064 nm), and depolarization profiles (532 and 1064 nm) in both nadir and zenith directions during long transects over the

  1. Aerosol composition and variability in the Baltimore-Washington, DC region

    NASA Astrophysics Data System (ADS)

    Beyersdorf, A. J.; Ziemba, L. D.; Chen, G.; Corr, C. A.; Crawford, J. H.; Diskin, G. S.; Moore, R. H.; Thornhill, K. L.; Winstead, E. L.; Anderson, B. E.

    2015-08-01

    In order to utilize satellite-based aerosol measurements for the determination of air quality, the relationship between aerosol optical properties (wavelength-dependent, column-integrated extinction measured by satellites) and mass measurements of aerosol loading (PM2.5 used for air quality monitoring) must be understood. This connection varies with many factors including those specific to the aerosol type, such as composition, size and hygroscopicity, and to the surrounding atmosphere, such as temperature, relative humidity (RH) and altitude, all of which can vary spatially and temporally. During the DISCOVER-AQ (Deriving Information on Surface conditions from Column and Vertically Resolved Observations Relevant to Air Quality) project, extensive in-situ atmospheric profiling in the Baltimore, MD-Washington, DC region was performed during fourteen flights in July 2011. Identical flight plans and profile locations throughout the project provide meaningful statistics for determining the variability in and correlations between aerosol loading, composition, optical properties and meteorological conditions. Measured water-soluble aerosol mass was composed primarily of ammonium sulfate (campaign average of 32 %) and organics (57 %). A distinct difference in composition was observed with high-loading days having a proportionally larger percentage of ammonium sulfate (up to 49 %) due to transport from the Ohio River Valley. This composition shift caused a change in the aerosol water-uptake potential (hygroscopicity) such that higher relative contributions of ammonium sulfate increased the bulk aerosol hygroscopicity. These days also tended to have higher relative humidity causing an increase in the water content of the aerosol. Conversely, low aerosol loading days had lower ammonium sulfate and higher black carbon contributions causing lower single scattering albedos (SSAs). The average black carbon concentrations were 240 ng m-3 in the lowest 1 km decreasing to 35 ng m-3

  2. Climate Impacts of CALIPSO-Guided Corrections to Black Carbon Aerosol Vertical Distributions in a Global Climate Model

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kovilakam, Mahesh; Mahajan, Salil; Saravanan, R.

    Here, we alleviate the bias in the tropospheric vertical distribution of black carbon aerosols (BC) in the Community Atmosphere Model (CAM4) using the Cloud-Aerosol and Infrared Pathfinder Satellite Observations (CALIPSO)-derived vertical profiles. A suite of sensitivity experiments are conducted with 1x, 5x, and 10x the present-day model estimated BC concentration climatology, with (corrected, CC) and without (uncorrected, UC) CALIPSO-corrected BC vertical distribution. The globally averaged top of the atmosphere radiative flux perturbation of CC experiments is ~8–50% smaller compared to uncorrected (UC) BC experiments largely due to an increase in low-level clouds. The global average surface temperature increases, the globalmore » average precipitation decreases, and the ITCZ moves northward with the increase in BC radiative forcing, irrespective of the vertical distribution of BC. Further, tropical expansion metrics for the poleward extent of the Northern Hemisphere Hadley cell (HC) indicate that simulated HC expansion is not sensitive to existing model biases in BC vertical distribution.« less

  3. Climate Impacts of CALIPSO-Guided Corrections to Black Carbon Aerosol Vertical Distributions in a Global Climate Model

    DOE PAGES

    Kovilakam, Mahesh; Mahajan, Salil; Saravanan, R.; ...

    2017-09-13

    Here, we alleviate the bias in the tropospheric vertical distribution of black carbon aerosols (BC) in the Community Atmosphere Model (CAM4) using the Cloud-Aerosol and Infrared Pathfinder Satellite Observations (CALIPSO)-derived vertical profiles. A suite of sensitivity experiments are conducted with 1x, 5x, and 10x the present-day model estimated BC concentration climatology, with (corrected, CC) and without (uncorrected, UC) CALIPSO-corrected BC vertical distribution. The globally averaged top of the atmosphere radiative flux perturbation of CC experiments is ~8–50% smaller compared to uncorrected (UC) BC experiments largely due to an increase in low-level clouds. The global average surface temperature increases, the globalmore » average precipitation decreases, and the ITCZ moves northward with the increase in BC radiative forcing, irrespective of the vertical distribution of BC. Further, tropical expansion metrics for the poleward extent of the Northern Hemisphere Hadley cell (HC) indicate that simulated HC expansion is not sensitive to existing model biases in BC vertical distribution.« less

  4. Assessment of 1D and 3D model simulated radiation flux based on surface measurements and estimation of aerosol forcing and their climatological aspects

    NASA Astrophysics Data System (ADS)

    Subba, T.; Gogoi, M. M.; Pathak, B.; Ajay, P.; Bhuyan, P. K.; Solmon, F.

    2018-05-01

    Ground reaching solar radiation flux was simulated using a 1-dimensional radiative transfer (SBDART) and a 3-dimensional regional climate (RegCM 4.4) model and their seasonality against simultaneous surface measurements carried out using a CNR4 net Radiometer over a sub-Himalayan foothill site of south-east Asia was assessed for the period from March 2013-January 2015. The model simulated incoming fluxes showed a very good correlation with the measured values with correlation coefficient R2 0.97. The mean bias errors between these two varied from -40 W m-2 to +7 W m-2 with an overestimation of 2-3% by SBDART and an underestimation of 2-9% by RegCM. Collocated measurements of the optical parameters of aerosols indicated a reduction in atmospheric transmission path by 20% due to aerosol load in the atmosphere when compared with the aerosol free atmospheric condition. Estimation of aerosol radiative forcing efficiency (ARFE) indicated that the presence of black carbon (BC, 10-15%) led to a surface dimming by -26.14 W m-2 τ-1 and a potential atmospheric forcing of +43.04 W m-2 τ-1. BC alone is responsible for >70% influence with a major role in building up of forcing efficiency of +55.69 W m-2 τ-1 (composite) in the atmosphere. On the other hand, the scattering due to aerosols enhance the outgoing radiation at the top of the atmosphere (ARFETOA -12.60 W m-2 ω-1), the absence of which would have resulted in ARFETOA of +16.91 W m-2 τ-1 (due to BC alone). As a result, 3/4 of the radiation absorption in the atmosphere is ascribed to the presence of BC. This translated to an atmospheric heating rate of 1.0 K day-1, with 0.3 K day-1 heating over the elevated regions (2-4 km) of the atmosphere, especially during pre-monsoon season. Comparison of the satellite (MODIS) derived and ground based estimates of surface albedo showed seasonal difference in their magnitudes (R2 0.98 during retreating monsoon and winter; 0.65 during pre-monsoon and monsoon), indicating that the

  5. Model-Based Estimation of Sampling-Caused Uncertainty in Aerosol Remote Sensing for Climate Research Applications

    NASA Technical Reports Server (NTRS)

    Geogdzhayev, Igor V.; Cairns, Brian; Mishchenko, Michael I.; Tsigaridis, Kostas; van Noije, Twan

    2014-01-01

    To evaluate the effect of sampling frequency on the global monthly mean aerosol optical thickness (AOT), we use 6 years of geographical coordinates of Moderate Resolution Imaging Spectroradiometer (MODIS) L2 aerosol data, daily global aerosol fields generated by the Goddard Institute for Space Studies General Circulation Model and the chemical transport models Global Ozone Chemistry Aerosol Radiation and Transport, Spectral Radiationtransport Model for Aerosol Species and Transport Model 5, at a spatial resolution between 1.125 deg × 1.125 deg and 2 deg × 3?: the analysis is restricted to 60 deg S-60 deg N geographical latitude. We found that, in general, the MODIS coverage causes an underestimate of the global mean AOT over the ocean. The long-term mean absolute monthly difference between all and dark target (DT) pixels was 0.01-0.02 over the ocean and 0.03-0.09 over the land, depending on the model dataset. Negative DT biases peak during boreal summers, reaching 0.07-0.12 (30-45% of the global long-term mean AOT). Addition of the Deep Blue pixels tempers the seasonal dependence of the DT biases and reduces the mean AOT difference over land by 0.01-0.02. These results provide a quantitative measure of the effect the pixel exclusion due to cloud contamination, ocean sun-glint and land type has on the MODIS estimates of the global monthly mean AOT. We also simulate global monthly mean AOT estimates from measurements provided by pixel-wide along-track instruments such as the Aerosol Polarimetry Sensor and the Cloud-Aerosol LiDAR with Orthogonal Polarization. We estimate the probable range of the global AOT standard error for an along-track sensor to be 0.0005-0.0015 (ocean) and 0.0029-0.01 (land) or 0.5-1.2% and 1.1-4% of the corresponding global means. These estimates represent errors due to sampling only and do not include potential retrieval errors. They are smaller than or comparable to the published estimate of 0.01 as being a climatologically significant

  6. East Asian Studies of Tropospheric Aerosols and their Impact on Regional Climate (EAST -AIRC): An overview

    NASA Technical Reports Server (NTRS)

    Zhangqing, Li; Li, C.; Chen, H.; Tsay, S.-C.; Holben, B.; Huang, J.; Li, B.; Maring, H.; Qian, Y.; Shi, G.; hide

    2011-01-01

    As the most populated region of the world, Asia is a major source of aerosols with potential large impact over vast downstream areas, Papers published in this special section describe the variety of aerosols observed in China and their effects and interactions with the regional climate as part of the East Asian Study of Tropospheric Aerosols and their Impact on Regional Climate (EAST-AIRC), The majority of the papers are based on analyses of observations made under three field projects, namely, the Atmospheric Radiation Measurements (ARM) Mobile Facility mission in China (AMF-China), the East Asian Study of Tropospheric Aerosols: An International Regional Experiment (EAST-AIRE), and the Atmospheric Aerosols of China and their Climate Effects (AACCE), The former two are U,S,-China collaborative projects, and the latter is a part of the China's National Basic Research program (or often referred to as "973 project"), Routine meteorological data of China are also employed in some studies, The wealth of general and speCIalized measurements lead to extensive and close-up investigations of the optical, physical, and chemical properties of anthropogenic, natural, and mixed aerosols; their sources, formation, and transport mechanisms; horizontal, vertical, and temporal variations; direct and indirect effects; and interactions with the East Asian monsoon system, Particular efforts are made to advance our understanding of the mixing and interaction between dust and anthropogenic pollutants during transport. Several modeling studies were carried out to simulate aerosol impact on radiation budget, temperature, precipitation, wind and atmospheric circulation, fog, etc, In addition, impacts of the Asian monsoon system on aerosol loading are also simulated.

  7. Recent Rainfall and Aerosol Chemistry From Bermuda

    NASA Astrophysics Data System (ADS)

    Landing, W. M.; Shelley, R.; Kadko, D. C.

    2014-12-01

    This project was devoted to testing the use of Be-7 as a tracer for quantifying trace element fluxes from the atmosphere to the oceans. Rainfall and aerosol samples were collected between June 15, 2011 and July 27, 2013 at the Bermuda Institute of Ocean Sciences (BIOS) located near the eastern end of the island of Bermuda. Collectors were situated near ground level, clear of surrounding vegetation, at a meteorological monitoring station in front of the BIOS laboratory, about 10 m above sea level. This is a Bermuda Air Quality Program site used for ambient air quality monitoring. To quantify the atmospheric deposition of Be-7, plastic buckets were deployed for collection of fallout over ~3 week periods. Wet deposition was collected for trace element analysis using a specially modified "GEOTRACES" N-CON automated wet deposition collector. Aerosol samples were collected with a Tisch TE-5170V-BL high volume aerosol sampler, modified to collect 12 replicate samples on acid-washed 47mm diameter Whatman-41 filters, using procedures identical to those used for the US GEOTRACES aerosol program (Morton et al., 2013). Aerosol and rainfall samples were analyzed for total Na, Mg, Al, P, Sc, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, Zn, Rb, Sr, Zr, Cd, Sb, Ba, La, Ce, Nd, Pb, Th, and U using ICPMS. Confirming earlier data from Bermuda, strong seasonality in rainfall and aerosol loading and chemistry was observed, particularly for aerosol and rainfall Fe concentrations when Saharan dust arrives in July/August with SE trajectories.

  8. Aerosol indirect effect on tropospheric ozone via lightning

    NASA Astrophysics Data System (ADS)

    Yuan, Tianle; Remer, Lorraine A.; Bian, Huisheng; Ziemke, Jerald R.; Albrecht, Rachel; Pickering, Kenneth E.; Oreopoulos, Lazaros; Goodman, Steven J.; Yu, Hongbin; Allen, Dale J.

    2012-09-01

    projecting future tropospheric O3forcing as well as wildfire changes and call for integrated investigations of the coupled aerosol-cloud-chemistry system.

  9. Aerosol indirect effect on tropospheric ozone via lightning

    NASA Astrophysics Data System (ADS)

    Yuan, T.; Remer, L. A.; Bian, H.; Ziemke, J. R.; Albrecht, R. I.; Pickering, K. E.; Oreopoulos, L.; Goodman, S. J.; Yu, H.; Allen, D. J.

    2012-12-01

    for understanding past and projecting future tropospheric O3 forcing as well as wildfire changes and call for integrated investigations of the coupled aerosol-cloud-chemistry system.

  10. Using the OMI Aerosol Index and Absorption Aerosol Optical Depth to evaluate the NASA MERRA Aerosol Reanalysis

    NASA Astrophysics Data System (ADS)

    Buchard, V.; da Silva, A. M.; Colarco, P. R.; Darmenov, A.; Randles, C. A.; Govindaraju, R.; Torres, O.; Campbell, J.; Spurr, R.

    2014-12-01

    A radiative transfer interface has been developed to simulate the UV Aerosol Index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and Aerosol Absorption Optical Depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of Aerosol Optical Depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the Aerosol Robotic Network (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the South African and South American biomass burning regions indicates that revising the spectrally-dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons

  11. Using the OMI aerosol index and absorption aerosol optical depth to evaluate the NASA MERRA Aerosol Reanalysis

    NASA Astrophysics Data System (ADS)

    Buchard, V.; da Silva, A. M.; Colarco, P. R.; Darmenov, A.; Randles, C. A.; Govindaraju, R.; Torres, O.; Campbell, J.; Spurr, R.

    2015-05-01

    A radiative transfer interface has been developed to simulate the UV aerosol index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and aerosol absorption optical depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the AErosol RObotic NETwork (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model-produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the southern African and South American biomass burning regions indicates that revising the spectrally dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons

  12. Assessment of the impact of forest fires on aerosols distribution in the atmosphere over Kyiv based on AERONET and satellites measurement techniques

    NASA Astrophysics Data System (ADS)

    Galytska, Evgenia; Danylevsky, Vassyl; Snizhko, Sergiy

    2015-04-01

    The study of the dynamics of aerosol particles, revealing their sources in the atmosphere is one of the urgent problems of modern meteorology, climatology, atmospheric physics, and ecology. Monitoring of the air pollution caused by aerosols contributes to the determination of its effects on the climate and to the reduction of its negative impacts on the health of the population. The research work comprises latest technologies and approaches: remote ground-based together with satellite measurements of the optical properties of aerosol particles, atmospheric dynamics research and modeling of transport of particles. The dynamics of aerosol layer properties over Ukrainian cities as Kyiv, Sevastopol, and over the rural site Martova is the subject of the remote sensing investigation made by the sun photometers network AERONET/PHOTONS, dealing with the columnar aerosol optical properties particularly aerosol optical depth (AOD). As well the CALIOP lidar data on board of CALIPSO satellite were used for AOD analysis for appropriate territory and further comparison with AERONET measurements. It was stated that during warm periods a large concentration of impurities was observed due to natural sources, such as forest fires in Ukraine and the European Russia. Especially in summer 2010 the high-altitude anticyclone and a ridge above the European Russia and Ural caused the hottest weather in the East Europe region for the period that promoted origin of vast and intensive forest fires in Central and Western Russia that caused reach pollution of the atmosphere over Ukraine by aerosols. Thus, in August 15, 2010 an aerosol optical depth over Kyiv at a wavelength of 440 nm reached a value of 1.5, which was associated with the aerosols arrival from these fires. Thus, the values of aerosol optical depth that date was triple more in comparison to usual distribution. The ways of aerosols arrival to the atmosphere over Kyiv from the fires centers during some days of August 2010 and effect

  13. Multi-Decadal Variation of Aerosols: Sources, Transport, and Climate Effects

    NASA Technical Reports Server (NTRS)

    Chin, Mian; Diehl, Thomas; Bian, Huisheng; Streets, David

    2008-01-01

    We present a global model study of multi-decadal changes of atmospheric aerosols and their climate effects using a global chemistry transport model along with the near-term to longterm data records. We focus on a 27-year time period of satellite era from 1980 to 2006, during which a suite of aerosol data from satellite observations, ground-based measurements, and intensive field experiments have become available. We will use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model, which involves a time-varying, comprehensive global emission dataset that we put together in our previous investigations and will be improved/extended in this project. This global emission dataset includes emissions of aerosols and their precursors from fuel combustion, biomass burning, volcanic eruptions, and other sources from 1980 to the present. Using the model and satellite data, we will analyze (1) the long-term global and regional aerosol trends and their relationship to the changes of aerosol and precursor emissions from anthropogenic and natural sources, (2) the intercontinental source-receptor relationships controlled by emission, transport pathway, and climate variability.

  14. Tennessee Valley Total and Cloud-to-Ground Lightning Climatology Comparison

    NASA Technical Reports Server (NTRS)

    Buechler, Dennis; Blakeslee, R. J.; Hall, J. M.; McCaul, E. W.

    2008-01-01

    The North Alabama Lightning Mapping Array (NALMA) has been in operation since 2001 and consists often VHF receivers deployed across northern Alabama. The NALMA locates sources of impulsive VHF radio signals from total lightning by accurately measuring the time that the signals arrive at the different receiving stations. The sources detected are then clustered into flashes by applying spatially and temporally constraints. This study examines the total lightning climatology of the region derived from NALMA and compares it to the cloud-to-ground (CG) climatology derived from the National Lightning Detection Network (NLDN) The presentation compares the total and CG lightning trends for monthly, daily, and hourly periods.

  15. Aerosols and their Impact on Radiation, Clouds, Precipitation & Severe Weather Events

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Li, Zhanqing; Rosenfeld, Daniel; Fan, Jiwen

    Aerosols, the tiny particles suspended in the atmosphere, have been in the forefront of environmental and climate change sciences as the primary atmospheric pollutant and external force affecting Earth’s weather and climate. There are two dominant mechanisms by which aerosols affect weather and climate: aerosol-radiation interactions (ARI) and aerosol-cloud interactions (ACI). ARI arises from aerosol scattering and absorption, which alters the radiation budgets of the atmosphere and surface, while ACI is rooted to the fact that aerosols serve as cloud condensation nuclei and ice nuclei. Both ARI and ACI are coupled with atmospheric dynamics to produce a chain of complexmore » interactions with a large range of meteorological variables that influence both weather and climate. Elaborated here are the impacts of aerosols on the radiation budget, clouds (microphysics, structure, and lifetime), precipitation, and severe weather events (lightning, thunderstorms, hail, and tornados). Depending on environmental variables and aerosol properties, the effects can be both positive and negative, posing the largest uncertainties in the external forcing of the climate system. This has considerably hindered our ability in projecting future climate changes and in doing accurate numerical weather predictions.« less

  16. Development, Comparisons and Evaluation of Aerosol Retrieval Algorithms

    NASA Astrophysics Data System (ADS)

    de Leeuw, G.; Holzer-Popp, T.; Aerosol-cci Team

    2011-12-01

    The Climate Change Initiative (cci) of the European Space Agency (ESA) has brought together a team of European Aerosol retrieval groups working on the development and improvement of aerosol retrieval algorithms. The goal of this cooperation is the development of methods to provide the best possible information on climate and climate change based on satellite observations. To achieve this, algorithms are characterized in detail as regards the retrieval approaches, the aerosol models used in each algorithm, cloud detection and surface treatment. A round-robin intercomparison of results from the various participating algorithms serves to identify the best modules or combinations of modules for each sensor. Annual global datasets including their uncertainties will then be produced and validated. The project builds on 9 existing algorithms to produce spectral aerosol optical depth (AOD and Ångström exponent) as well as other aerosol information; two instruments are included to provide the absorbing aerosol index (AAI) and stratospheric aerosol information. The algorithms included are: - 3 for ATSR (ORAC developed by RAL / Oxford university, ADV developed by FMI and the SU algorithm developed by Swansea University ) - 2 for MERIS (BAER by Bremen university and the ESA standard handled by HYGEOS) - 1 for POLDER over ocean (LOA) - 1 for synergetic retrieval (SYNAER by DLR ) - 1 for OMI retreival of the absorbing aerosol index with averaging kernel information (KNMI) - 1 for GOMOS stratospheric extinction profile retrieval (BIRA) The first seven algorithms aim at the retrieval of the AOD. However, each of the algorithms used differ in their approach, even for algorithms working with the same instrument such as ATSR or MERIS. To analyse the strengths and weaknesses of each algorithm several tests are made. The starting point for comparison and measurement of improvements is a retrieval run for 1 month, September 2008. The data from the same month are subsequently used for

  17. Ultraviolet and visible radiation at Barrow, Alaska: Climatology and influencing factors on the basis of version 2 National Science Foundation network data

    NASA Astrophysics Data System (ADS)

    Bernhard, Germar; Booth, Charles R.; Ehramjian, James C.; Stone, Robert; Dutton, Ellsworth G.

    2007-05-01

    Spectral ultraviolet (UV) and visible irradiance has been measured near Barrow, Alaska (71°N, 157°W), between 1991 and 2005 with a SUV-100 spectroradiometer. The instrument is part of the U.S. National Science Foundation's UV Monitoring Network. Here we present results based on the recently produced "version 2" data release, which supersedes published "version 0" data. Cosine error and wavelength-shift corrections applied to the new version increased biologically effective UV dose rates by 0-10%. Corrected clear-sky measurements of different years are typically consistent to within ±3%. Measurements were complemented with radiative transfer model calculations to retrieve total ozone and surface albedo from measured spectra and for the separation of the different factors influencing UV and visible radiation. A climatology of UV and visible radiation was established, focusing on annual cycles, trends, and the effect of clouds. During several episodes in spring of abnormally low total ozone, the daily UV dose at 305 nm exceeded the climatological mean by up to a factor of 2.6. Typical noontime UV Indices during summer vary between 2 and 4; the highest UV Index measured was 5.0 and occurred when surface albedo was unusually high. Radiation levels in the UV-A and visible exhibit a strong spring-autumn asymmetry. Irradiance at 345 nm peaks on approximately 20 May, 1 month before the solstice. This asymmetry is caused by increased cloudiness in autumn and high albedo in spring, when the snow covered surface enhances downwelling UV irradiance by up to 57%. Clouds reduce UV radiation at 345 nm on average by 4% in March and by more than 40% in August. Aerosols reduce UV by typically 5%, but larger reductions were observed during Arctic haze events. Stratospheric aerosols from the Pinatubo eruption in 1991 enhanced spectral irradiance at 305 nm for large solar zenith angles. The year-to-year variations of spectral irradiance at 305 nm and of the UV Index are mostly caused

  18. Analysis of global land surface albedo climatology and spatial-temporal variation during 1981-2010 from multiple satellite products

    NASA Astrophysics Data System (ADS)

    He, Tao; Liang, Shunlin; Song, Dan-Xia

    2014-09-01

    For several decades, long-term time series data sets of multiple global land surface albedo products have been generated from satellite observations. These data sets have been used as one of the key variables in climate change studies. This study aims to assess the surface albedo climatology and to analyze long-term albedo changes, from nine satellite-based data sets for the period 1981-2010, on a global basis. Results show that climatological surface albedo data sets derived from satellite observations can be used to validate, calibrate, and further improve surface albedo simulations and parameterizations in current climate models. However, the albedo products derived from the International Satellite Cloud Climatology Project and the Global Energy and Water Exchanges Project have large seasonal biases. At latitudes higher than 50°, the maximal difference in winter zonal albedo ranges from 0.1 to 0.4 among the nine satellite data sets. Satellite-based albedo data sets agree relatively well during the summer at high latitudes, with a standard deviation of 0.04 for the 70°-80° zone in both hemispheres. The fine-resolution (0.05°) data sets agree well with each other for all the land cover types in middle to low latitudes; however, large spread was identified for their albedos at middle to high latitudes over land covers with mixed snow and sparse vegetation. By analyzing the time series of satellite-based albedo products over the past three decades, albedo of the Northern Hemisphere was found to be decreasing in July, likely due to the shrinking snow cover. Meanwhile, albedo in January was found to be increasing, likely because of the expansion of snow cover in northern winter. However, to improve the albedo estimation at high latitudes, and ultimately the climate models used for long-term climate change studies, a still better understanding of differences between satellite-based albedo data sets is required.

  19. Importance of including ammonium sulfate ((NH4)2SO4) aerosols for ice cloud parameterization in GCMs

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bhattacharjee, P. S.; Sud, Yogesh C.; Liu, Xiaohong

    2010-02-22

    A common deficiency of many cloud-physics parameterizations including the NASA’s microphysics of clouds with aerosol- cloud interactions (hereafter called McRAS-AC) is that they simulate less (larger) than the observed ice cloud particle number (size). A single column model (SCM) of McRAS-AC and Global Circulation Model (GCM) physics together with an adiabatic parcel model (APM) for ice-cloud nucleation (IN) of aerosols were used to systematically examine the influence of ammonium sulfate ((NH4)2SO4) aerosols, not included in the present formulations of McRAS-AC. Specifically, the influence of (NH4)2SO4 aerosols on the optical properties of both liquid and ice clouds were analyzed. First anmore » (NH4)2SO4 parameterization was included in the APM to assess its effect vis-à-vis that of the other aerosols. Subsequently, several evaluation tests were conducted over the ARM-SGP and thirteen other locations (sorted into pristine and polluted conditions) distributed over marine and continental sites with the SCM. The statistics of the simulated cloud climatology were evaluated against the available ground and satellite data. The results showed that inclusion of (NH4)2SO4 in the SCM made a remarkable improvement in the simulated effective radius of ice clouds. However, the corresponding ice-cloud optical thickness increased more than is observed. This can be caused by lack of cloud advection and evaporation. We argue that this deficiency can be mitigated by adjusting the other tunable parameters of McRAS-AC such as precipitation efficiency. Inclusion of ice cloud particle splintering introduced through well- established empirical equations is found to further improve the results. Preliminary tests show that these changes make a substantial improvement in simulating the cloud optical properties in the GCM, particularly by simulating a far more realistic cloud distribution over the ITCZ.« less

  20. Simulated CONUS Flash Flood Climatologies from Distributed Hydrologic Models

    NASA Astrophysics Data System (ADS)

    Flamig, Z.; Gourley, J. J.; Vergara, H. J.; Kirstetter, P. E.; Hong, Y.

    2016-12-01

    This study will describe a CONUS flash flood climatology created over the period from 2002 through 2011. The MRMS reanalysis precipitation dataset was used as forcing into the Ensemble Framework For Flash Flood Forecasting (EF5). This high resolution 1-sq km 5-minute dataset is ideal for simulating flash floods with a distributed hydrologic model. EF5 features multiple water balance components including SAC-SMA, CREST, and a hydrophobic model all coupled with kinematic wave routing. The EF5/SAC-SMA and EF5/CREST water balance schemes were used for the creation of dual flash flood climatologies based on the differing water balance principles. For the period from 2002 through 2011 the daily maximum streamflow, unit streamflow, and time of peak streamflow was stored along with the minimum soil moisture. These variables are used to describe the states of the soils right before a flash flood event and the peak streamflow that was simulated during the flash flood event. The results will be shown, compared and contrasted. The resulting model simulations will be verified on basins less than 1,000-sq km with USGS gauges to ensure the distributed hydrologic models are reliable. The results will also be compared spatially to Storm Data flash flood event observations to judge the degree of agreement between the simulated climatologies and observations.

  1. Informing Aerosol Transport Models With Satellite Multi-Angle Aerosol Measurements

    NASA Technical Reports Server (NTRS)

    Limbacher, J.; Patadia, F.; Petrenko, M.; Martin, M. Val; Chin, M.; Gaitley, B.; Garay, M.; Kalashnikova, O.; Nelson, D.; Scollo, S.

    2011-01-01

    As the aerosol products from the NASA Earth Observing System's Multi-angle Imaging SpectroRadiometer (MISR) mature, we are placing greater focus on ways of using the aerosol amount and type data products, and aerosol plume heights, to constrain aerosol transport models. We have demonstrated the ability to map aerosol air-mass-types regionally, and have identified product upgrades required to apply them globally, including the need for a quality flag indicating the aerosol type information content, that varies depending upon retrieval conditions. We have shown that MISR aerosol type can distinguish smoke from dust, volcanic ash from sulfate and water particles, and can identify qualitative differences in mixtures of smoke, dust, and pollution aerosol components in urban settings. We demonstrated the use of stereo imaging to map smoke, dust, and volcanic effluent plume injection height, and the combination of MISR and MODIS aerosol optical depth maps to constrain wildfire smoke source strength. This talk will briefly highlight where we stand on these application, with emphasis on the steps we are taking toward applying the capabilities toward constraining aerosol transport models, planet-wide.

  2. Intercomparison between CMIP5 model and MODIS satellite-retrieved data of aerosol optical depth, cloud fraction, and cloud-aerosol interactions

    NASA Astrophysics Data System (ADS)

    Sockol, Alyssa; Small Griswold, Jennifer D.

    2017-08-01

    Aerosols are a critical component of the Earth's atmosphere and can affect the climate of the Earth through their interactions with solar radiation and clouds. Cloud fraction (CF) and aerosol optical depth (AOD) at 550 nm from the Moderate Resolution Imaging Spectroradiometer (MODIS) are used with analogous cloud and aerosol properties from Historical Phase 5 of the Coupled Model Intercomparison Project (CMIP5) model runs that explicitly include anthropogenic aerosols and parameterized cloud-aerosol interactions. The models underestimate AOD by approximately 15% and underestimate CF by approximately 10% overall on a global scale. A regional analysis is then used to evaluate model performance in two regions with known biomass burning activity and absorbing aerosol (South America (SAM) and South Africa (SAF)). In SAM, the models overestimate AOD by 4.8% and underestimate CF by 14%. In SAF, the models underestimate AOD by 35% and overestimate CF by 13.4%. Average annual cycles show that the monthly timing of AOD peaks closely match satellite data in both SAM and SAF for all except the Community Atmosphere Model 5 and Geophysical Fluid Dynamics Laboratory (GFDL) models. Monthly timing of CF peaks closely match for all models (except GFDL) for SAM and SAF. Sorting monthly averaged 2° × 2.5° model or MODIS CF as a function of AOD does not result in the previously observed "boomerang"-shaped CF versus AOD relationship characteristic of regions with absorbing aerosols from biomass burning. Cloud-aerosol interactions, as observed using daily (or higher) temporal resolution data, are not reproducible at the spatial or temporal resolution provided by the CMIP5 models.

  3. Assessment of the aerosol distribution over Indian subcontinent in CMIP5 models

    NASA Astrophysics Data System (ADS)

    Sanap, S. D.; Ayantika, D. C.; Pandithurai, G.; Niranjan, K.

    2014-04-01

    This paper examines the aerosol distribution over Indian subcontinent as represented in 21 models from Coupled Model Inter-comparison Project Phase 5 (CMIP5) simulations, wherein model simulated aerosol optical depth (AOD) is compared with Moderate Resolution Imaging Spectro-radiometer (MODIS) satellite observations. The objective of the study is to provide an assessment of the capability of various global models, participating in CMIP5 project, in capturing the realistic spatial and temporal distribution of aerosol species over the Indian subcontinent. Results from our analysis show that majority of the CMIP5 models (excepting HADGEM2-ES, HADGEM2-CC) seriously underestimates the spatio-temporal variability of aerosol species over the Indian subcontinent, in particular over Indo-Gangetic Plains (IGP). Since IGP region is dominated by anthropogenic activities, high population density, and wind driven transport of dust and other aerosol species, MODIS observations reveal high AOD values over this region. Though the representation of black carbon (BC) loading in many models is fairly good, the dust loading is observed to be significantly low in majority of the models. The presence of pronounced dust activity over northern India and dust being one of the major constituent of aerosol species, the biases in dust loading has a great impact on the AOD of that region. We found that considerable biases in simulating the 850 hPa wind field (which plays important role in transport of dust from adjacent deserts) would be the possible reason for poor representation of dust AOD and in turn total AOD over Indian region in CMIP5 models. In addition, aerosol radiative forcing (ARF) underestimated/overestimated in most of the models. However, spatial distribution of ARF in multi-model ensemble mean is comparable reasonably well with observations with bias in magnitudes. This analysis emphasizes the fundamental need to improve the representation of aerosol species in current state of

  4. Biology of the Coarse Aerosol Mode: Insights Into Urban Aerosol Ecology

    NASA Astrophysics Data System (ADS)

    Dueker, E.; O'Mullan, G. D.; Montero, A.

    2015-12-01

    Microbial aerosols have been understudied, despite implications for climate studies, public health, and biogeochemical cycling. Because viable bacterial aerosols are often associated with coarse aerosol particles, our limited understanding of the coarse aerosol mode further impedes our ability to develop models of viable bacterial aerosol production, transport, and fate in the outdoor environment, particularly in crowded urban centers. To address this knowledge gap, we studied aerosol particle biology and size distributions in a broad range of urban and rural settings. Our previously published findings suggest a link between microbial viability and local production of coarse aerosols from waterways, waste treatment facilities, and terrestrial systems in urban and rural environments. Both in coastal Maine and in New York Harbor, coarse aerosols and viable bacterial aerosols increased with increasing wind speeds above 4 m s-1, a dynamic that was observed over time scales ranging from minutes to hours. At a New York City superfund-designated waterway regularly contaminated with raw sewage, aeration remediation efforts resulted in significant increases of coarse aerosols and bacterial aerosols above that waterway. Our current research indicates that bacterial communities in aerosols at this superfund site have a greater similarity to bacterial communities in the contaminated waterway with wind speeds above 4 m s-1. Size-fractionated sampling of viable microbial aerosols along the urban waterfront has also revealed significant shifts in bacterial aerosols, and specifically bacteria associated with coarse aerosols, when wind direction changes from onshore to offshore. This research highlights the key connections between bacterial aerosol viability and the coarse aerosol fraction, which is important in assessments of production, transport, and fate of bacterial contamination in the urban environment.

  5. Measurements of Semi-volatile Aerosol and Its Effect on Aerosol Optical Properties During Southern Oxidant and Aerosol Study

    NASA Astrophysics Data System (ADS)

    Khlystov, A.; Grieshop, A. P.; Saha, P.; Subramanian, R.

    2013-12-01

    Semi-volatile compounds, including particle-bound water, comprise a large part of aerosol mass and have a significant influence on aerosol lifecycle and its optical properties. Understanding the properties of semi-volatile compounds, especially those pertaining to gas/aerosol partitioning, is of critical importance for our ability to predict concentrations and properties of ambient aerosol. A set of state-of-the-art instruments was deployed at the SEARCH site near Centerville, AL during the Southern Oxidant and Aerosol Study (SOAS) campaign in summer 2013 to measure the effect of temperature and relative humidity on aerosol size distribution, composition and optical properties. Light scattering and absorption by temperature- and humidity-conditioned aerosols was measured using three photo-acoustic extinctiometers (PAX) at three wavelengths (405 nm, 532 nm, and 870 nm). In parallel to these measurements, a long residence time temperature-stepping thermodenuder and a variable residence time constant temperature thermodenuder in combination with three SMPS systems and an Aerosol Chemical Speciation Monitor (ACSM) were used to assess aerosol volatility and kinetics of aerosol evaporation. It was found that both temperature and relative humidity have a strong effect on aerosol optical properties. The variable residence time thermodenuder data suggest that aerosol equilibrated fairly quickly, within 2 s, in contrast to other ambient observations. Preliminary analysis show that approximately 50% and 90% of total aerosol mass evaporated at temperatures of 100 C and 180C, respectively. Evaporation varied substantially with ambient aerosol loading and composition and meteorology. During course of this study, T50 (temperatures at which 50% aerosol mass evaporates) varied from 60 C to more than 120 C.

  6. Improving Aerosol and Visibility Forecasting Capabilities Using Current and Future Generations of Satellite Observations

    DTIC Science & Technology

    2015-08-27

    Shi et al. (2011) suggested that large spatial discrepancies exist in operational satellite aerosol products such as MODIS and MISR. Thus, before...to be fully evaluated. In the past few years of the project period, MODIS Deep Blue (DB) and MISR aerosol products have been studied, and schemes for...constructing DA-grade MODIS DB and MISR aerosol products have been developed and transitioned to the Naval Research Laboratory (NRL). Continuing

  7. Dust, Pollution, and Biomass Burning Aerosols in Asian Pacific: A Column Satellite-Surface Perspective

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee

    2004-01-01

    Airborne dusts from northern China contribute a significant part of the air quality problem and, to some extent, regional climatic impact in Asia during spring-time. However, with the economical growth in China, increases in the emission of air pollutants generated from industrial and vehicular sources will not only impact the radiation balance, but adverse health effects to humans all year round. In addition, both of these dust and air pollution clouds can transport swiftly across the Pacific reaching North America within a few days, possessing an even larger scale effect. The Asian dust and air pollution aerosols can be detected by its colored appearance on current Earth observing satellites (e.g., MODIS, SeaWiFS, TOMS, etc.) and its evolution monitored by satellites and surface network. Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially those in Africa, South America, and Southeast Asia. However, the unique climatology of Southeast Asia is very different than that of Africa and South America, such that large-scale biomass burning causes smoke to interact extensively with clouds during the peak-burning season of March to April. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass burning processes. These gases influence the Earth-atmosphere system, impacting both global climate and tropospheric chemistry. Some aerosols can serve as cloud condensation nuclei, which play an important role in determining cloud lifetime and precipitation, hence, altering the earth's radiation and water budget. Biomass burning also affects the biogeochemical cycling of nitrogen and carbon compounds from the soil to the atmosphere; the hydrological cycle (i.e., run off and evaporation); land surface reflectivity and emissivity; as well as ecosystem biodiversity and stability. Two new initiatives, EAST-AIRE (East

  8. Sensitive study of the climatological SST by using ATSR global SST data sets

    NASA Astrophysics Data System (ADS)

    Xue, Yong; Lawrence, Sean P.; Llewellyn-Jones, David T.

    1995-12-01

    Climatological sea surface temperature (SST) is an initial step for global climate processing monitoring. A comparison has been made by using Oberhuber's SST data set and two years monthly averaged SST from ATSR thermal band data to force the OGCM. In the eastern Pacific Ocean, these make only a small difference to model SST. In the western Pacific Ocean, the use of Oberhuber's data set gives higher climatological SST than that using ATSR data. The SSTs were also simulated for 1992 using climatological SSTs from two years monthly averaged ATSR data and Oberhuber data. The forcing with SST from ATSR data was found to give better SST simulation than that from Oberhuber's data. Our study has confirmed that ATSR can provide accurate monthly averaged global SST for global climate processing monitoring.

  9. AerChemMIP: Quantifying the effects of chemistry and aerosols in CMIP6

    DOE PAGES

    Collins, William J.; Lamarque, Jean -François; Schulz, Michael; ...

    2017-02-09

    The Aerosol Chemistry Model Intercomparison Project (AerChemMIP) is endorsed by the Coupled-Model Intercomparison Project 6 (CMIP6) and is designed to quantify the climate and air quality impacts of aerosols and chemically reactive gases. These are specifically near-term climate forcers (NTCFs: methane, tropospheric ozone and aerosols, and their precursors), nitrous oxide and ozone-depleting halocarbons. The aim of AerChemMIP is to answer four scientific questions. 1. How have anthropogenic emissions contributed to global radiative forcing and affected regional climate over the historical period? 2. How might future policies (on climate, air quality and land use) affect the abundances of NTCFs and theirmore » climate impacts? 3.How do uncertainties in historical NTCF emissions affect radiative forcing estimates? 4. How important are climate feedbacks to natural NTCF emissions, atmospheric composition, and radiative effects? These questions will be addressed through targeted simulations with CMIP6 climate models that include an interactive representation of tropospheric aerosols and atmospheric chemistry. These simulations build on the CMIP6 Diagnostic, Evaluation and Characterization of Klima (DECK) experiments, the CMIP6 historical simulations, and future projections performed elsewhere in CMIP6, allowing the contributions from aerosols and/or chemistry to be quantified. As a result, specific diagnostics are requested as part of the CMIP6 data request to highlight the chemical composition of the atmosphere, to evaluate the performance of the models, and to understand differences in behaviour between them.« less

  10. AerChemMIP: Quantifying the effects of chemistry and aerosols in CMIP6

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Collins, William J.; Lamarque, Jean -François; Schulz, Michael

    The Aerosol Chemistry Model Intercomparison Project (AerChemMIP) is endorsed by the Coupled-Model Intercomparison Project 6 (CMIP6) and is designed to quantify the climate and air quality impacts of aerosols and chemically reactive gases. These are specifically near-term climate forcers (NTCFs: methane, tropospheric ozone and aerosols, and their precursors), nitrous oxide and ozone-depleting halocarbons. The aim of AerChemMIP is to answer four scientific questions. 1. How have anthropogenic emissions contributed to global radiative forcing and affected regional climate over the historical period? 2. How might future policies (on climate, air quality and land use) affect the abundances of NTCFs and theirmore » climate impacts? 3.How do uncertainties in historical NTCF emissions affect radiative forcing estimates? 4. How important are climate feedbacks to natural NTCF emissions, atmospheric composition, and radiative effects? These questions will be addressed through targeted simulations with CMIP6 climate models that include an interactive representation of tropospheric aerosols and atmospheric chemistry. These simulations build on the CMIP6 Diagnostic, Evaluation and Characterization of Klima (DECK) experiments, the CMIP6 historical simulations, and future projections performed elsewhere in CMIP6, allowing the contributions from aerosols and/or chemistry to be quantified. As a result, specific diagnostics are requested as part of the CMIP6 data request to highlight the chemical composition of the atmosphere, to evaluate the performance of the models, and to understand differences in behaviour between them.« less

  11. Los Alamos Climatology 2016 Update

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bruggeman, David Alan

    The Los Alamos National Laboratory (LANL or the Laboratory) operates a meteorology monitoring network to support LANL emergency response, engineering designs, environmental compliance, environmental assessments, safety evaluations, weather forecasting, environmental monitoring, research programs, and environmental restoration. Weather data has been collected in Los Alamos since 1910. Bowen (1990) provided climate statistics (temperature and precipitation) for the 1961– 1990 averaging period, and included other analyses (e.g., wind and relative humidity) based on the available station locations and time periods. This report provides an update to the 1990 publication Los Alamos Climatology (Bowen 1990).

  12. The Derivation Of A CO2 Fugacity Climatology From SOCAT's Global In SITU Data

    NASA Astrophysics Data System (ADS)

    Goddijn-Murphy, L. M.; Woolf, D. K.; Land, P. E.; Shutler, J. D.

    2013-12-01

    The Surface Ocean CO2 Atlas (SOCAT) has made millions of global underway sea surface measurements of CO2 publicly available, all in a uniform format and presented as fugacity, fCO2. However, these fCO2 values are valid strictly only for the instantaneous temperature at measurement and are not ideal for climatology. We recomputed these fCO2 values for the measurement month to be applicable to climatological sea surface temperatures, extrapolated to reference year 2010. The data were then spatially interpolated on a 1°×1° grid of the global oceans to produce 12 monthly fCO2 distributions. Our climatology data will be shared with the science community.

  13. A satellite and model based flood inundation climatology of Australia

    NASA Astrophysics Data System (ADS)

    Schumann, G.; Andreadis, K.; Castillo, C. J.

    2013-12-01

    To date there is no coherent and consistent database on observed or simulated flood event inundation and magnitude at large scales (continental to global). The only compiled data set showing a consistent history of flood inundation area and extent at a near global scale is provided by the MODIS-based Dartmouth Flood Observatory. However, MODIS satellite imagery is only available from 2000 and is hampered by a number of issues associated with flood mapping using optical images (e.g. classification algorithms, cloud cover, vegetation). Here, we present for the first time a proof-of-concept study in which we employ a computationally efficient 2-D hydrodynamic model (LISFLOOD-FP) complemented with a sub-grid channel formulation to generate a complete flood inundation climatology of the past 40 years (1973-2012) for the entire Australian continent. The model was built completely from freely available SRTM-derived data, including channel widths, bank heights and floodplain topography, which was corrected for vegetation canopy height using a global ICESat canopy dataset. Channel hydraulics were resolved using actual channel data and bathymetry was estimated within the model using hydraulic geometry. On the floodplain, the model simulated the flow paths and inundation variables at a 1 km resolution. The developed model was run over a period of 40 years and a floodplain inundation climatology was generated and compared to satellite flood event observations. Our proof-of-concept study demonstrates that this type of model can reliably simulate past flood events with reasonable accuracies both in time and space. The Australian model was forced with both observed flow climatology and VIC-simulated flows in order to assess the feasibility of a model-based flood inundation climatology at the global scale.

  14. Biomass-burning Aerosols in South East-Asia: Smoke Impact Assessment(BASE-ASIA)

    NASA Technical Reports Server (NTRS)

    Tsay, Si-Chee; Hsu, Christina N.; King, Michael D.; Shu, Peter K.

    2002-01-01

    Biomass burning has been a regular practice for land clearing and land conversion in many countries, especially in Africa, South America, and South East Asia. Significant global sources of greenhouse gases (e.g., CO2, CH4), chemically active gases (e.g., NO, CO, HC, CH3Br), and atmospheric aerosols are produced by biomass-burning processes, which influence the Earth-atmosphere energetics and hence impact both global climate and tropospheric chemistry. Some gases and aerosols can serve as active cloud condensation nuclei, which play important role in determining the net radiation budget, precipitation rate, and cloud lifetime. Biomass burning also affects the biogeochemical cycling of nitrogen and carbon compounds from the soil to the atmosphere; the hydrological cycle (i.e., run off and evaporation); the reflectivity and emissivity of the land; and the stability of ecosystems and ecosystem biodiversity. Compared to Africa and South America, the climatology in South East Asia reveals quite different characteristics, showing distinct large-scale smoke and cloud sources and interaction regimes. The fresh water distribution in this region is highly dependent on monsoon rainfall; in fact, the predictability of the tropical climate system is much reduced during the boreal spring, which is associated with the peak season of biomass burning activities. Estimating the burning fuel (e.g., bark, branches, and wood), an important part of studying regional carbon cycle, may rely on utilizing a wide range of distinctive spectral features in the shortwave and longwave regions. Therefore, to accurately assess the impact of smoke aerosols in this region requires continuous observations from satellites, aircraft, networks of ground-based instruments and dedicated field experiments. A new initiative will be proposed and discussed.

  15. Laboratory studies of stratospheric aerosol chemistry

    NASA Technical Reports Server (NTRS)

    Molina, Mario J.

    1996-01-01

    In this report we summarize the results of the two sets of projects funded by the NASA grant NAG2-632, namely investigations of various thermodynamic and nucleation properties of the aqueous acid system which makes up stratospheric aerosols, and measurements of reaction probabilities directly on ice aerosols with sizes corresponding to those of polar stratospheric cloud particles. The results of these investigations are of importance for the assessment of the potential stratospheric effects of future fleets of supersonic aircraft. In particular, the results permit to better estimate the effects of increased amounts of water vapor and nitric acid (which forms from nitrogen oxides) on polar stratospheric clouds and on the chemistry induced by these clouds.

  16. The Effect of Aerosol Hygroscopicity and Volatility on Aerosol Optical Properties During Southern Oxidant and Aerosol Study

    NASA Astrophysics Data System (ADS)

    Khlystov, A.; Grieshop, A. P.; Saha, P.; Subramanian, R.

    2014-12-01

    Secondary organic aerosol (SOA) from biogenic sources can influence optical properties of ambient aerosol by altering its hygroscopicity and contributing to light absorption directly via formation of brown carbon and indirectly by enhancing light absorption by black carbon ("lensing effect"). The magnitude of these effects remains highly uncertain. A set of state-of-the-art instruments was deployed at the SEARCH site near Centerville, AL during the Southern Oxidant and Aerosol Study (SOAS) campaign in summer 2013 to measure the effect of relative humidity and temperature on aerosol size distribution, composition and optical properties. Light scattering and absorption by temperature- and humidity-conditioned aerosols was measured using three photo-acoustic extinctiometers (PAX) at three wavelengths (405 nm, 532 nm, and 870 nm). The sample-conditioning system provided measurements at ambient RH, 10%RH ("dry"), 85%RH ("wet"), and 200 C ("TD"). In parallel to these measurements, a long residence time temperature-stepping thermodenuder (TD) and a variable residence time constant temperature TD in combination with three SMPS systems and an Aerosol Chemical Speciation Monitor (ACSM) were used to assess aerosol volatility and kinetics of aerosol evaporation. We will present results of the on-going analysis of the collected data set. We will show that both temperature and relative humidity have a strong effect on aerosol optical properties. SOA appears to increase aerosol light absorption by about 10%. TD measurements suggest that aerosol equilibrated fairly quickly, within 2 s. Evaporation varied substantially with ambient aerosol loading and composition and meteorology.

  17. Aerosol characterizaton in El Paso-Juarez airshed using optical methods

    NASA Astrophysics Data System (ADS)

    Esparza, Angel Eduardo

    2011-12-01

    The assessment and characterization of atmospheric aerosols and their optical properties are of great significance for several applications such as air pollution studies, atmospheric visibility, remote sensing of the atmosphere, and impacts on climate change. Decades ago, the interest in atmospheric aerosols was primarily for visibility impairment problems; however, recently interest has intensified with efforts to quantify the optical properties of aerosols, especially because of the uncertainties surrounding the role of aerosols in climate change. The main objective of the optical characterization of aerosols is to understand their properties. These properties are determined by the aerosols' chemical composition, size, shape and concentration. The general purpose of this research was to contribute to a better characterization of the aerosols present in the Paso del Norte Basin. This study permits an alternative approach in the understanding of air pollution for this zone by analyzing the predominant components and their contributions to the local environment. This dissertation work had three primary objectives, in which all three are intertwined by the general purpose of the aerosol characterization in the Paso del Norte region. The first objective was to retrieve the columnar aerosol size distribution for two different cases (clean and polluted scenarios) at each season (spring, summer, fall and winter) of the year 2009. In this project, instruments placed in buildings within the University of Texas at El Paso (UTEP) as well as a monitoring site (CAMS 12) from the Texas Commission on Environmental Quality (TCEQ) provided the measurements that delimited the aerosol size distribution calculated by our model, the Environmental Physics Inverse Reconstruction (EPIRM) model. The purpose of this objective was to provide an alternate method of quantifying and size-allocating aerosols in situ, by using the optical properties of the aerosols and inversely reconstruct and

  18. Understanding of the Regional Aerosol Characterization over the North-eastern part of the Indian Subcontinent: South-Asian Region

    NASA Astrophysics Data System (ADS)

    Dahutia, P.; Pathak, B.

    2016-12-01

    The north-eastern region (NER) of India is a part of Indian subcontinent owing a unique topography surrounded by three sides by high mountain and open in the west. The long-term characterization of aerosol and its effect on climate is carried out in 11 locations over NER of India along with two adjoining locations Dhaka (DAC) and Banmauk (BNK) (22-30°N and 88-98°E) using multiple satellite retrievals and model data. Quality assured monthly Level 3 Collection 6 data of MODerate Resolution Imaging Spectroradiometer (MODIS) data retrieved from both Aqua and Terra having 1°×1° resolution of columnar Aerosol Optical Depth (AOD) and its associated parameters for the period of 2001-2014. Investigation revealed a distinct spatio-temporal variation over all the locations with highest climatological mean AOD in Dhaka (0.66±0.19) and lowest in high altitude location Thimphu (0.17±0.1). The parameter Absorbing aerosols Index (AAI) from combine TOMS and OMI instrument is used to study absorbing aerosols during 1979-2014. The seasonal AOD and AAI are highest during pre-monsoon months while lowest in retreating monsoon in all the locations. The continuous wavelet transform (CWT) analysis of non-smoothen time-series of AOD revealed the strong annual oscillation (AO) of total columnar aerosol loading. The annual trend analysis of aerosol parameters shows a statistically significant (i.e., p<0.05) increasing trends of AOD ( 0.009-0.001year-1) as well as AAI ( 0.015-0.001year-1) over all locations. The simultaneous increase in Angtröm Exponent (AE) along with AOD and AAI indicates the enhancement of anthropogenic aerosols which might have a contribution to the climate change. The performed long-term (1979-2014) regression analysis of seasonal and annual mean of Net Surface Downward Shortwave Flux (NSDSF), Cloud Optical Depth (COD), rainfall and temperature shows a signature of climate change over this region. The opposite trend of COD (increasing) and NSDSF (decreasing

  19. Comment on "'Elevated Heat Pump' Hypothesis for the Aerosol-Monsoon Hydroclimate Link: 'Grounded' in Observations?" by S. Nigam and M. Bollasina

    NASA Technical Reports Server (NTRS)

    Lau, K. M.; Kim, K. M.

    2011-01-01

    In their recent paper, Nigam and Bollasina [2010] (hereinafter NB) claimed to have found observational evidences that are at variance with the elevated heat pump (EHP) hypothesis regarding the possible impacts of absorbing aerosols on the South Asian summer monsoon [Lau et al., 2006; Lau and Kim, 2006]. We found NB's arguments and inferences against the EHP hypothesis flawed, stemming from their own out of context interpretation of the hypothesis. NB argued that the simultaneous negative correlation of aerosol with rainfall, and correlations with other quantities in May, are evidence against the EHP hypothesis. Their argument cannot be justified. First, Lau and Kim [2006] (hereinafter LK06) never stated that the main rainfall response to EHP is in May. Second, the EHP is about responses of the entire Indian monsoon system that are nonlocal in space and time with respect to the aerosol forcing. As shown in Figure 4 of LK06, while the aerosol anomalies are strongest in April-May, the strongest rainfall response is in June-July, with the enhanced rainfall fed by an induced thermally driven circulation which brings additional moisture from the ocean to the Indian subcontinent. Third, the increased rainfall over the Bay of Bengal as shown in Figure 1a of NB and the increased low-level convergence in Figure 1f of NB do not necessarily reflect responses associated with EHP but rather the large ]scale circulation that provides the buildup of the aerosols before the onset of the monsoon rainfall over India. Because aerosol can only accumulate where there is little or no washout by rain, the negative correlation is a necessary condition for increased atmospheric loading of aerosols. For the same reason, the spatial distributions of rainfall and aerosol generally are offset with each other, i.e., high aerosol in regions of low rainfall. This is evident in Figure 1, which shows the climatological mean of the MODIS aerosol optical depth (AOD), and TRMM rainfall over India in

  20. Aerosol effect on climate extremes in Europe under different future scenarios

    NASA Astrophysics Data System (ADS)

    Sillmann, J.; Pozzoli, L.; Vignati, E.; Kloster, S.; Feichter, J.

    2013-05-01

    This study investigates changes in extreme temperature and precipitation events under different future scenarios of anthropogenic aerosol emissions (i.e., SO2 and black and organic carbon) simulated with an aerosol-climate model (ECHAM5-HAM) with focus on Europe. The simulations include a maximum feasible aerosol reduction (MFR) scenario and a current legislation emission (CLEmod) scenario where Europe implements the MFR scenario, but the rest of the world follows the current legislation scenario and a greenhouse gas scenario. The strongest changes relative to the year 2000 are projected for the MFR scenario, in which the global aerosol reduction greatly enforces the general warming effect due to greenhouse gases and results in significant increases of temperature and precipitation extremes in Europe. Regional warming effects can also be identified from aerosol reductions under the CLEmodscenario. This becomes most obvious in the increase of the hottest summer daytime temperatures in Northern Europe.

  1. Interactive coupling of regional climate and sulfate aerosol models over eastern Asia

    NASA Astrophysics Data System (ADS)

    Qian, Yun; Giorgi, Filippo

    1999-03-01

    The NCAR regional climate model (RegCM) is interactively coupled to a simple radiatively active sulfate aerosol model over eastern Asia. Both direct and indirect aerosol effects are represented. The coupled model system is tested for two simulation periods, November 1994 and July 1995, with aerosol sources representative of present-day anthropogenic sulfur emissions. The model sensitivity to the intensity of the aerosol source is also studied. The main conclusions from our work are as follows: (1) The aerosol distribution and cycling processes show substantial regional spatial variability, and temporal variability varying on a range of scales, from the diurnal scale of boundary layer and cumulus cloud evolution to the 3-10 day scale of synoptic scale events and the interseasonal scale of general circulation features; (2) both direct and indirect aerosol forcings have regional effects on surface climate; (3) the regional climate response to the aerosol forcing is highly nonlinear, especially during the summer, due to the interactions with cloud and precipitation processes; (4) in our simulations the role of the aerosol indirect effects is dominant over that of direct effects; (5) aerosol-induced feedback processes can affect the aerosol burdens at the subregional scale. This work constitutes the first step in a long term research project aimed at coupling a hierarchy of chemistry/aerosol models to the RegCM over the eastern Asia region.

  2. Dust transport over the eastern Mediterranean derived from Total Ozone Mapping Spectrometer, Aerosol Robotic Network, and surface measurements

    NASA Astrophysics Data System (ADS)

    Kalivitis, N.; Gerasopoulos, E.; Vrekoussis, M.; Kouvarakis, G.; Kubilay, N.; Hatzianastassiou, N.; Vardavas, I.; Mihalopoulos, N.

    2007-02-01

    Multiyear surface PM10 measurements performed on Crete Island, Greece, have been used in conjunction with satellite (Total Ozone Mapping Spectrometer (TOMS)) and ground-based remote sensing measurements (Aerosol Robotic Network (AERONET)) to enhance our understanding of the evolution of mineral dust events over the eastern Mediterranean. An analysis of southerly air masses at altitudes of 1000 and 3000 m over a 5 year period (2000-2005), showed that dust can potentially arrive over Crete, either simultaneously in the lower free troposphere and inside the boundary layer (vertical extended transport (VET)) or initially into the free troposphere with the heavier particles gradually being scavenged inside the boundary layer (free troposphere transport (FTT)). Both pathways present significant seasonal variations but on an annual basis contribute almost equally to the dust transport in the area. During VET the aerosol index (AI) derived from TOMS was significantly correlated with surface PM10, and in general AI was found to be adequate for the characterization of dust loadings over the eastern Mediterranean on a climatological basis. A significant covariance between PM10 and AOT was observed during VET as well, indicating that AOT levels from AERONET may be estimated by PM10 levels at the surface. Surface measurements are thus crucial for the validation of remote sensing measurements and hence are a powerful tool for the investigation of the impact of aerosols on climate.

  3. Coupling Satellite and Ground-Based Instruments to Map Climate Forcing by Anthropogenic Aerosols

    NASA Technical Reports Server (NTRS)

    Charlson, Robert J.; Anderson, Theodore L.; Hostetler, Chris (Technical Monitor)

    2000-01-01

    Climate forcing by anthropogenic aerosols is a significant but highly uncertain factor in global climate change. Only satellites can offer the global coverage essential to reducing this uncertainty; however, satellite measurements must be coupled with correlative, in situ measurements both to constrain the aerosol optical properties required in satellite retrieval algorithms and to provide chemical identification of aerosol sources. This grant funded the first two years of a three-year project which seeks to develop methodologies for combining spaceborne lidar with in-situ aerosol data sets to improve estimates of direct aerosol climate forcing. Progress under this two-year grant consisted in the development and deployment of a new in-situ capability for measuring aerosol 180' backscatter and the extinction-to-backscatter ratio. This new measurement capacity allows definitive lidar/in-situ comparisons and improves our ability to interpret lidar data in terms of climatically relevant quantities such as the extinction coefficient and optical depth. Measurements were made along the coast of Washington State, in Central Illinois, over the Indian Ocean, and in the Central Pacific. Thus, this research, combined with previous measurements by others, is rapidly building toward a global data set of extinction-to-backscatter ratio for key aerosol types. Such information will be critical to interpreting lidar data from the upcoming PICASSO-CENA, or P-C, satellite mission. Another aspect of this project is to investigate innovative ways to couple the lidar-satellite signal with targeted in-situ measurements toward a direct determination of aerosol forcing. This aspect is progressing in collaboration with NASA Langley's P-C lidar simulator and radiative transfer modeling by the University of Lille, France.

  4. Coupling Satellite and Ground-Based Instruments to Map Climate Forcing by Anthropogenic Aerosol

    NASA Technical Reports Server (NTRS)

    Charlson, Robert J.; Anderson, Theodore L.; Hostetler, Chris (Technical Monitor)

    2000-01-01

    Climate forcing by anthropogenic aerosols is a significant but highly uncertain factor in global climate change. Only satellites can offer the global coverage essential to reducing this uncertainty; however, satellite measurements must be coupled with correlative, in situ measurements both to constrain the aerosol optical properties required in satellite retrieval algorithms and to provide chemical identification of aerosol sources. This grant funded the third year of a three-year project which seeks to develop methodologies for combining spaceborne lidar with in-situ aerosol data sets to improve estimates of direct aerosol climate forcing. Progress under this one-year grant consisted in analysis and publication of field studies using a new in-situ capability for measuring aerosol 180 deg backscatter and the extinction-to-backscatter ratio. This new measurement capacity allows definitive lidar/in-situ comparisons and improves our ability to interpret lidar data in terms of climatically relevant quantities such as the extinction coefficient and optical depth. Analyzed data consisted of measurements made along the coast of Washington State, in Central Illinois, over the Indian Ocean, and in the Central Pacific. Thus, this research, combined with previous measurements by others, is rapidly building toward a global data set of extinction-to-backscatter ratio for key aerosol types. Such information will be critical to interpreting lidar data from the upcoming PICASSO-CENA, or P-C, satellite mission. Another aspect of this project is to investigate innovative ways to couple the lidar-satellite signal with target in-situ measurements toward a direct determination of aerosol forcing. This aspect is progressing in collaboration with NASA Langley's P-C lidar simulator.

  5. Aerosols, Chemistry, and Radiative Forcing: A 3-D Model Analysis of Satellite and ACE-Asia data (ACMAP)

    NASA Technical Reports Server (NTRS)

    Chin, Mian; Ginoux, Paul; Torres, Omar; Zhao, Xue-Peng

    2005-01-01

    We propose a research project to incorporate a global 3-D model and satellite data into the multi-national Aerosol Characterization Experiment-Asia (ACE-Asia) mission. Our objectives are (1) to understand the physical, chemical, and optical properties of aerosols and the processes that control those properties over the Asian-Pacific region, (2) to investigate the interaction between aerosols and tropospheric chemistry, and (3) to determine the aerosol radiative forcing over the Asia-Pacific region. We will use the Georgia TecWGoddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model to link satellite observations and the ACE-Asia measurements. First, we will use the GOCART model to simulate aerosols and related species, and evaluate the model with satellite and in-situ observations. Second, the model generated aerosol vertical profiles and compositions will be used to validate the satellite products; and the satellite data will be used for during- and post- mission analysis. Third, we will use the model to analyze and interpret both satellite and ACE- Asia field campaign data and investigate the aerosol-chemistry interactions. Finally, we will calculate aerosol radiative forcing over the Asian-Pacific region, and assess the influence of Asian pollution in the global atmosphere. We propose a research project to incorporate a global 3-D model and satellite data into

  6. Tower Mesonetwork Climatology and Interactive Display Tool

    NASA Technical Reports Server (NTRS)

    Case, Jonathan L.; Bauman, William H., III

    2004-01-01

    Forecasters at the 45th Weather Squadron and Spaceflight Meteorology Group use data from the tower network over the Kennedy Space Center (KSC) and Cape Canaveral Air Force Station (CCAFS) to evaluate Launch Commit Criteria, and issue and verify forecasts for ground operations. Systematic biases in these parameters could adversely affect an analysis, forecast, or verification. Also, substantial geographical variations in temperature and wind speed can occur under specific wind directions. To address these concerns, the Applied Meteorology Unit (AMU) developed a climatology of temperatures and winds from the tower network, and identified the geographical variation and significant tower biases. The mesoclimate is largely driven by the complex land-water interfaces across KSC/CCAFS. Towers with close proximity to water typically had much warmer nocturnal temperatures and higher wind speeds throughout the year. The strongest nocturnal wind speeds occurred from October to March whereas the strongest mean daytime wind speeds occurred from February to May. These results of this project can be viewed by forecasters through an interactive graphical user interface developed by the AMU. The web-based interface includes graphical and map displays of mean, standard deviation, bias, and data availability for any combination of towers, variables, months, hours, and wind directions.

  7. Development of the Multi-Angle Stratospheric Aerosol Radiometer (MASTAR) Instrument

    NASA Astrophysics Data System (ADS)

    DeLand, M. T.; Colarco, P. R.; Kowalewski, M. G.; Gorkavyi, N.; Ramos-Izquierdo, L.

    2017-12-01

    Aerosol particles in the stratosphere ( 15-25 km altitude), both produced naturally and perturbed by volcanic eruptions and anthropogenic emissions, continue to be a source of significant uncertainty in the Earth's energy budget. Stratospheric aerosols can offset some of the warming effects caused by greenhouse gases. These aerosols are currently monitored using measurements from the Ozone Mapping and Profiling Suite (OMPS) Limb Profiler (LP) instrument on the Suomi NPP satellite. In order to improve the sensitivity and spatial coverage of these aerosol data, we are developing an aerosol-focused compact version of the OMPS LP sensor called Multi-Angle Stratospheric Aerosol Radiometer (MASTAR) to fly on a 3U Cubesat satellite, using a NASA Instrument Incubator Program (IIP) grant. This instrument will make limb viewing measurements of the atmosphere in multiple directions simultaneously, and uses only a few selected wavelengths to reduce size and cost. An initial prototype version has been constructed using NASA GSFC internal funding and tested in the laboratory. Current design work is targeted towards a preliminary field test in Spring 2018. We will discuss the scientific benefits of MASTAR and the status of the project.

  8. A comparison of cirrus clouds determined by ISCCP and SAGE-II and their relation to convection in the tropics

    NASA Technical Reports Server (NTRS)

    Christopher, Sundar A.; Vonder Haar, Thomas H.

    1992-01-01

    Results of tropical thin cirrus cloud retrievals using International Satellite Cloud Climatology Project (ISCCP) and Stratospheric Aerosol and Gaseous Experiment (SAGE-II) data from January 1985 are presented. A preliminary analysis of the results shows that thin cirrus increases with increasing height in both data sets, and SAGE-II exhibits a high frequency of occurrence. The thin cirrus extinction coefficient shows maxima around the convective regions of South America and the western Pacific Ocean.

  9. Strong Constraints on Aerosol-Cloud Interactions from Volcanic Eruptions

    NASA Technical Reports Server (NTRS)

    Malavelle, Florent F.; Haywood, Jim M.; Jones, Andy; Gettelman, Andrew; Clarisse, Lieven; Bauduin, Sophie; Allan, Richard P.; Karset, Inger Helene H.; Kristjansson, Jon Egill; Oreopoulos, Lazaros; hide

    2017-01-01

    Aerosols have a potentially large effect on climate, particularly through their interactions with clouds, but the magnitude of this effect is highly uncertain. Large volcanic eruptions produce sulfur dioxide, which in turn produces aerosols; these eruptions thus represent a natural experiment through which to quantify aerosol-cloud interactions. Here we show that the massive 2014-2015 fissure eruption in Holuhraun, Iceland, reduced the size of liquid cloud droplets - consistent with expectations - but had no discernible effect on other cloud properties. The reduction in droplet size led to cloud brightening and global-mean radiative forcing of around minus 0.2 watts per square metre for September to October 2014. Changes in cloud amount or cloud liquid water path, however, were undetectable, indicating that these indirect effects, and cloud systems in general, are well buffered against aerosol changes. This result will reduce uncertainties in future climate projections, because we are now able to reject results from climate models with an excessive liquid-water-path response.

  10. Strong constraints on aerosol-cloud interactions from volcanic eruptions.

    PubMed

    Malavelle, Florent F; Haywood, Jim M; Jones, Andy; Gettelman, Andrew; Clarisse, Lieven; Bauduin, Sophie; Allan, Richard P; Karset, Inger Helene H; Kristjánsson, Jón Egill; Oreopoulos, Lazaros; Cho, Nayeong; Lee, Dongmin; Bellouin, Nicolas; Boucher, Olivier; Grosvenor, Daniel P; Carslaw, Ken S; Dhomse, Sandip; Mann, Graham W; Schmidt, Anja; Coe, Hugh; Hartley, Margaret E; Dalvi, Mohit; Hill, Adrian A; Johnson, Ben T; Johnson, Colin E; Knight, Jeff R; O'Connor, Fiona M; Partridge, Daniel G; Stier, Philip; Myhre, Gunnar; Platnick, Steven; Stephens, Graeme L; Takahashi, Hanii; Thordarson, Thorvaldur

    2017-06-22

    Aerosols have a potentially large effect on climate, particularly through their interactions with clouds, but the magnitude of this effect is highly uncertain. Large volcanic eruptions produce sulfur dioxide, which in turn produces aerosols; these eruptions thus represent a natural experiment through which to quantify aerosol-cloud interactions. Here we show that the massive 2014-2015 fissure eruption in Holuhraun, Iceland, reduced the size of liquid cloud droplets-consistent with expectations-but had no discernible effect on other cloud properties. The reduction in droplet size led to cloud brightening and global-mean radiative forcing of around -0.2 watts per square metre for September to October 2014. Changes in cloud amount or cloud liquid water path, however, were undetectable, indicating that these indirect effects, and cloud systems in general, are well buffered against aerosol changes. This result will reduce uncertainties in future climate projections, because we are now able to reject results from climate models with an excessive liquid-water-path response.

  11. Configuration and Assessment of the GISS ModelE2 Contributions to the CMIP5 Archive

    NASA Technical Reports Server (NTRS)

    Schmidt, Gavin A.; Kelley, Max; Nazarenko, Larissa; Ruedy, Reto; Russell, Gary L.; Aleinov, Igor; Bauer, Mike; Bauer, Susanne E.; Bhat, Maharaj K.; Bleck, Rainer; hide

    2014-01-01

    We present a description of the ModelE2 version of the Goddard Institute for Space Studies (GISS) General Circulation Model (GCM) and the configurations used in the simulations performed for the Coupled Model Intercomparison Project Phase 5 (CMIP5). We use six variations related to the treatment of the atmospheric composition, the calculation of aerosol indirect effects, and ocean model component. Specifically, we test the difference between atmospheric models that have noninteractive composition, where radiatively important aerosols and ozone are prescribed from precomputed decadal averages, and interactive versions where atmospheric chemistry and aerosols are calculated given decadally varying emissions. The impact of the first aerosol indirect effect on clouds is either specified using a simple tuning, or parameterized using a cloud microphysics scheme. We also use two dynamic ocean components: the Russell and HYbrid Coordinate Ocean Model (HYCOM) which differ significantly in their basic formulations and grid. Results are presented for the climatological means over the satellite era (1980-2004) taken from transient simulations starting from the preindustrial (1850) driven by estimates of appropriate forcings over the 20th Century. Differences in base climate and variability related to the choice of ocean model are large, indicating an important structural uncertainty. The impact of interactive atmospheric composition on the climatology is relatively small except in regions such as the lower stratosphere, where ozone plays an important role, and the tropics, where aerosol changes affect the hydrological cycle and cloud cover. While key improvements over previous versions of the model are evident, these are not uniform across all metrics.

  12. Climatology of Ultra Violet(UV) Irradiance at the Surface of the Earth as Measured by the Belgian UV Radiation Monitoring Network

    NASA Astrophysics Data System (ADS)

    Pandey, Praveen; Gillotay, Didier; Depiesse, Cedric

    2016-08-01

    In this paper we describe the network of ground-based ultraviolet (UV) radiation monitoring stations in Belgium. The evolution of the entire network, together with the details of measuring instruments is given. The observed cumulative irradiations -UVB, UVA and total solar irradiation (TSI)- over the course of measurement for three stations -a northern (Ostende), central (Uccle) and a southern (Redu)- are shown. The longest series of measurement shown in this study is at Uccle, Brussels, from 1995 till 2014. Thus, the variation of the UV index, together with the variation of irradiations during summer and winter months at Uccle are shown as a part of this climatological study. The trend of UVB irradiance over the above mentioned three stations is shown. This UVB trend is studied in conjunction with the long-term satellite-based total column ozone value over Belgium, which shows two distinct trends marked by a change point. The total column ozone trend following the change point is positive. It is also seen that the UVB trend is positive for the urban/sub-urban sites: Uccle and Redu. Whereas the UVB trend at Ostende, which is a coastal site, is not positive. A possible explanation of this relation between total column ozone and UVB trend could be associated with aerosols, which is shown in this paper by means of a radiative transfer model based study -as a part of a preliminary investigation. It is seen that the UVI is influenced by the type of aerosols.

  13. Imaging aerosol viscosity

    NASA Astrophysics Data System (ADS)

    Pope, Francis; Athanasiadis, Thanos; Botchway, Stan; Davdison, Nicholas; Fitzgerald, Clare; Gallimore, Peter; Hosny, Neveen; Kalberer, Markus; Kuimova, Marina; Vysniauskas, Aurimas; Ward, Andy

    2017-04-01

    Organic aerosol particles play major roles in atmospheric chemistry, climate, and public health. Aerosol particle viscosity is important since it can determine the ability of chemical species such as oxidants, organics or water to diffuse into the particle bulk. Recent measurements indicate that OA may be present in highly viscous states; however, diffusion rates of small molecules such as water appear not to be limited by these high viscosities. We have developed a technique for measuring viscosity that allows for the imaging of aerosol viscosity in micron sized aerosols through use of fluorescence lifetime imaging of viscosity sensitive dyes which are also known as 'molecular rotors'. These rotors can be introduced into laboratory generated aerosol by adding minute quantities of the rotor to aerosol precursor prior to aerosolization. Real world aerosols can also be studied by doping them in situ with the rotors. The doping is achieved through generation of ultrafine aerosol particles that contain the rotors; the ultrafine aerosol particles deliver the rotors to the aerosol of interest via impaction and coagulation. This work has been conducted both on aerosols deposited on microscope coverslips and on particles that are levitated in their true aerosol phase through the use of a bespoke optical trap developed at the Central Laser Facility. The technique allows for the direct observation of kinetic barriers caused by high viscosity and low diffusivity in aerosol particles. The technique is non-destructive thereby allowing for multiple experiments to be carried out on the same sample. It can dynamically quantify and track viscosity changes during atmospherically relevant processes such oxidation and hygroscopic growth (1). This presentation will focus on the oxidation of aerosol particles composed of unsaturated and saturated organic species. It will discuss how the type of oxidant, oxidation rate and the composition of the oxidized products affect the time

  14. CATS Cloud and Aerosol Level 2 Heritage Edition Data Products.

    NASA Astrophysics Data System (ADS)

    Rodier, S. D.; Vaughan, M.; Yorks, J. E.; Palm, S. P.; Selmer, P. A.; Hlavka, D. L.; McGill, M. J.; Trepte, C. R.

    2017-12-01

    The Cloud-Aerosol Transport System (CATS) instrument was developed at NASA's Goddard Space Flight Center (GSFC) and deployed to the International Space Station (ISS) in January 2015. The CATS elastic backscatter lidars have been operating continuously in one of two science modes since February 2015. One of the primary science objectives of CATS is to continue the CALIPSO aerosol and cloud profile data record to provide continuity of lidar climate observations during the transition from CALIPSO to EarthCARE. To accomplish this, the CATS project at NASA's Goddard Space Flight Center (GSFC) and the CALIPSO project at NASA's Langley Research Center (LaRC) closely collaborated to develop and deliver a full suite of CALIPSO-like level 2 data products using the latest version of the CALIPSO level 2 Version 4 algorithms for the CATS data acquired while operating in science mode 1 (Multi-beam backscatter detection at 1064 and 532 nm, with depolarization measurement at both wavelengths). In this work, we present the current status of the CATS Heritage (i.e. CALIPSO-like) level 2 data products derived from the recent released CATS Level 1B V2-08 data. Extensive comparisons are performed between the three data sets (CALIPSO V4.10 Level 2, CATS Level 2 Operational V2-00 and CATS Heritage V1.00) for cloud and aerosol measurements (e.g., cloud-top height cloud-phase, cloud-layer occurrence frequency and cloud-aerosol discrimination) along the ISS path. In addition, global comparisons (between 52°S and 52°N) of aerosol extinction profiles derived from the CATS Level 2 Operational products and CALIOP V4 Level 2 products are presented. Comparisons of aerosol optical depths retrieved from active sensors (CATS and CALIOP) and passive sensors (MODIS) will provide context for the extinction profile comparisons.

  15. Tibetan Plateau glacier and hydrological change under stratospheric aerosol injection

    NASA Astrophysics Data System (ADS)

    Ji, D.

    2017-12-01

    As an important inland freshwater resource, mountain glaciers are highly related to human life, they provide water for many large rivers and play a very important role in regional water cycles. The response of mountain glaciers to future climate change is a topic of concern especially to the many people who rely on glacier-fed rivers for purposes such as irrigation. Geoengineering by stratospheric aerosol injection is a method of offsetting the global temperature rise from greenhouse gases. How the geoengineering by stratospheric aerosol injection affects the mass balance of mountain glaciers and adjacent river discharge is little understood. In this study, we use regional climate model WRF and catchment-based river model CaMa-Flood to study the impacts of stratospheric aerosol injection to Tibetan Plateau glacier mass balance and adjacent river discharge. To facilitate mountain glacier mass balance study, we improve the description of mountain glacier in the land surface scheme of WRF. The improvements include: (1) a fine mesh nested in WRF horizontal grid to match the highly non-uniform spatial distribution of the mountain glaciers, (2) revising the radiation flux at the glacier surface considering the surrounding terrain. We use the projections of five Earth system models for CMIP5 rcp45 and GeoMIP G4 scenarios to drive the WRF and CaMa-Flood models. The G4 scenario, which uses stratospheric aerosols to reduce the incoming shortwave while applying the rcp4.5 greenhouse gas forcing, starts stratospheric sulfate aerosol injection at a rate of 5 Tg per year over the period 2020-2069. The ensemble projections suggest relatively slower glacier mass loss rates and reduced river discharge at Tibetan Plateau and adjacent regions under geoengineering scenario by stratospheric aerosol injection.

  16. Sampling Analysis of Aerosol Retrievals by Single-track Spaceborne Instrument for Climate Research

    NASA Astrophysics Data System (ADS)

    Geogdzhayev, I. V.; Cairns, B.; Alexandrov, M. D.; Mishchenko, M. I.

    2012-12-01

    We examine to what extent the reduced sampling of along-track instruments such as Cloud-Aerosol LIdar with Orthogonal Polarisation (CALIOP) and Aerosol Polarimetry Sensor (APS) affects the statistical accuracy of a satellite climatology of retrieved aerosol optical thickness (AOT) by sub-sampling the retrievals from a wide-swath imaging instrument (MODerate resolution Imaging Spectroradiometer (MODIS)). Owing to its global coverage, longevity, and extensive characterization versus ground based data, the MODIS level-2 aerosol product is an instructive testbed for assessing sampling effects on climatic means derived from along-track instrument data. The advantage of using daily pixel-level aerosol retrievals from MODIS is that limitations caused by the presence of clouds are implicit in the sample, so that their seasonal and regional variations are captured coherently. However, imager data can exhibit cross-track variability of monthly global mean AOTs caused by a scattering-angle dependence. We found that single along-track values can deviate from the imager mean by 15% over land and by more than 20% over ocean. This makes it difficult to separate natural variability from viewing-geometry artifacts complicating direct comparisons of an along-track sub-sample with the full imager data. To work around this problem, we introduce "flipped-track" sampling which, by design, is statistically equivalent to along-track sampling and while closely approximating the imager in terms of angular artifacts. We show that the flipped-track variability of global monthly mean AOT is much smaller than the cross-track one for the 7-year period considered. Over the ocean flipped-track standard error is 85% less than the cross-track one (absolute values 0.0012 versus 0.0079), and over land it is about one third of the cross-track value (0.0054 versus 0.0188) on average. This allows us to attribute the difference between the two errors to the viewing-geometry artifacts and obtain an upper

  17. Tourism climatology past and present: A review of the role of the ISB Commission on Climate, Tourism and Recreation.

    PubMed

    de Freitas, C R

    2017-09-01

    The Executive Board of the International Society of Biometeorology (ISB) founded the Commission on Climate, Tourism and Recreation (CCTR) at the 15th International Congress of Biometeorology in Sydney, Australia in 1999. The aims of the CCTR are to bring together researchers from around the world to critically review the current state of knowledge in tourism and recreation climatology and explore possibilities for future research. Almost two decades on, research in tourism climatology has developed and expanded due in large part to the initiatives and activities of the CCTR and several collaborative research projects run under the auspices of the CCTR. This work is reviewed here. Recent CCTR meeting highlighted the fact that, although climate is an essential part of the resource base for tourism, which is one of the world's biggest and fastest growing industries, relatively little is known about the effects of climate on tourist choices and broad demand patterns or the influence climate has on the commercial prospects and sustainability of tourism operators and destinations. The work here reviews what has been done, its conceptual underpinnings and current research frontiers.

  18. Regional and Global Aspects of Aerosols in Western Africa: From Air Quality to Climate

    NASA Technical Reports Server (NTRS)

    Chin, Mian; Diehl, Thomas; Kucsera, Tom; Spinhime, Jim; Palm, Stephen; Holben, Brent; Ginoux, Paul

    2006-01-01

    Western Africa is one of the most important aerosol source regions in the world. Major aerosol sources include dust from the world's largest desert Sahara, biomass burning from the Sahel, pollution aerosols from local sources and long-range transport from Europe, and biogenic sources from vegetation. Because these sources have large seasonal variations, the aerosol composition over the western Africa changes significantly with time. These aerosols exert large influences on local air quality and regional climate. In this study, we use the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model to analyze satellite lidar data from the GLAS instrument on the ICESat and the sunphotometer data from the ground-based network AERONET taken in both the wet (September - October 2003) and dry (February - March 2004) seasons over western Africa. We will quantify the seasonal variations of aerosol sources and compositions and aerosol spatial (horizontal and vertical) distributions over western Africa. We will also assess the climate impact of western African aerosols. Such studies will be applied to support the international project, Africa Monsoon Multidisciplinary Analysis (AMMA) and to analyze the AMMA data.

  19. Identifying Aerosol Type/Mixture from Aerosol Absorption Properties Using AERONET

    NASA Technical Reports Server (NTRS)

    Giles, D. M.; Holben, B. N.; Eck, T. F.; Sinyuk, A.; Dickerson, R. R.; Thompson, A. M.; Slutsker, I.; Li, Z.; Tripathi, S. N.; Singh, R. P.; hide

    2010-01-01

    Aerosols are generated in the atmosphere through anthropogenic and natural mechanisms. These sources have signatures in the aerosol optical and microphysical properties that can be used to identify the aerosol type/mixture. Spectral aerosol absorption information (absorption Angstrom exponent; AAE) used in conjunction with the particle size parameterization (extinction Angstrom exponent; EAE) can only identify the dominant absorbing aerosol type in the sample volume (e.g., black carbon vs. iron oxides in dust). This AAE/EAE relationship can be expanded to also identify non-absorbing aerosol types/mixtures by applying an absorption weighting. This new relationship provides improved aerosol type distinction when the magnitude of absorption is not equal (e.g, black carbon vs. sulfates). The Aerosol Robotic Network (AERONET) data provide spectral aerosol optical depth and single scattering albedo - key parameters used to determine EAE and AAE. The proposed aerosol type/mixture relationship is demonstrated using the long-term data archive acquired at AERONET sites within various source regions. The preliminary analysis has found that dust, sulfate, organic carbon, and black carbon aerosol types/mixtures can be determined from this AAE/EAE relationship when applying the absorption weighting for each available wavelength (Le., 440, 675, 870nm). Large, non-spherical dust particles absorb in the shorter wavelengths and the application of 440nm wavelength absorption weighting produced the best particle type definition. Sulfate particles scatter light efficiently and organic carbon particles are small near the source and aggregate over time to form larger less absorbing particles. Both sulfates and organic carbon showed generally better definition using the 870nm wavelength absorption weighting. Black carbon generation results from varying combustion rates from a number of sources including industrial processes and biomass burning. Cases with primarily black carbon showed

  20. Some Spatial Aspects of Southeastern United States Climatology.

    ERIC Educational Resources Information Center

    Soule, Peter T.

    1998-01-01

    Focuses on the climatology of an eight-state region in the southern and southeastern United States. Discusses general controls of climate and spatial patterns of various climatic averages. Examines mapped extremes as a means of fostering increased awareness of the variability that exists for climatic conditions in the region. (CMK)