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Sample records for atomic collision physics

  1. On the utility and ubiquity of atomic collision physics

    SciTech Connect

    Datz, S.

    1989-01-01

    This paper is divided into three parts. In the introduction, we discuss the history and makeup of ICPEAC. In the second part, we discuss the extent of applicability of atomic collision physics. In the third part, we chose one subject (dielectronic excitation) to show the interrelationship of various sub-branches of atomic collision physics. 28 refs., 14 figs.

  2. Sixteenth International Conference on the physics of electronic and atomic collisions

    SciTech Connect

    Dalgarno, A.; Freund, R.S.; Lubell, M.S.; Lucatorto, T.B.

    1989-01-01

    This report contains abstracts of papers on the following topics: photons, electron-atom collisions; electron-molecule collisions; electron-ion collisions; collisions involving exotic species; ion- atom collisions, ion-molecule or atom-molecule collisions; atom-atom collisions; ion-ion collisions; collisions involving rydberg atoms; field assisted collisions; collisions involving clusters and collisions involving condensed matter.

  3. Atomic collisions, inelastic indeed

    NASA Astrophysics Data System (ADS)

    Bercegol, Herve; Ferrando, Gwenael; Lehoucq, Roland

    At the turn of the twentieth century, a hot controversy raged about the ability of Boltzmann's framework to take care of irreversibility. The so-called Loschmidt's paradox progressively faded with time during the last hundred years, due to the predictive efficiency of statistical mechanics. However, one detail at the origin of the controversy - the elasticity of atomic collisions - was not completely challenged. A semi-classical treatment of two atoms interacting with the vacuum zero-point field permits to predict a friction force acting against the rotation of the pair of atoms. By its form and its level, the calculated torque is a candidate as a physical cause for diffusion of energy and angular momentum, and consequently for entropy growth. It opens the way to a revision of the standard vision of irreversibility. This presentation will focus on two points. First we will discuss the recent result in a broader context of electromagnetic interactions during microscopic collisions. The predicted friction phenomenon can be compared to and distinguished from Collision-Induced Emission and other types of inelastic collisions. Second we will investigate the consequences of the friction torque on calculated trajectories of colliding atoms, quantifying the generation of dimers linked by dispersion forces.

  4. Neutrino-atom collisions

    NASA Astrophysics Data System (ADS)

    Kouzakov, Konstantin A.; Studenikin, Alexander I.

    2016-05-01

    Neutrino-atom scattering provides a sensitive tool for probing nonstandard interactions of massive neutrinos in laboratory measurements. The ionization channel of this collision process plays an important role in experiments searching for neutrino magnetic moments. We discuss some theoretical aspects of atomic ionization by massive neutrinos. We also outline possible manifestations of neutrino electromagnetic properties in coherent elastic neutrino-nucleus scattering.

  5. Photonic, Electronic and Atomic Collisions

    NASA Astrophysics Data System (ADS)

    Fainstein, Pablo D.; Lima, Marco Aurelio P.; Miraglia, Jorge E.; Montenegro, Eduardo C.; Rivarola, Roberto D.

    2006-11-01

    -coincidence technique / T. Kaneyasu, T. Azuma and K. Okuno. Recent developments in proton-transfer-reaction mass spectrometry / A. Wisthaler ... [et al.]. Interferences in electron emission from H[symbol] induced by fast ions / N. Stolterfoht. Atomic realization of the young single electron interference process in individual autoionization collisions / R. O. Barrachina and M. Šitnik. Multiple ionization processes related to irradiation of biological tissue / M. E. Galassi ... [et al.]. Atom-diatom collisions at cold and ultra-cold temperatures / F. D. Colavecchia, G. A. Parker and R. T. Pack. Interactions of ions with hydrogen atoms / A. Luca, G. Borodi and D. Gerlich. Analysis of all structures in the elastic and charge transfer cross sections for proton-hydrogen collisions in the range of 10[symbol]-10øeV / P. S. Krstić ... [et al.]. Ab-initio ion-atom collision calculations for many-electron systems / J. Anton and B. Fricke. Fully differential studies on single ionization of helium by slow proton impact / A. Hasan ... [et al.]. Dipole polarization effects on highly-charged-ion-atom electron capture / C. C. Havener ... [et al.]. Proton-, antiproton-, and photon-he collisions in the context of ultra fast processes / T. Morishita ... [et al.]. Impact parameter dependent charge exchange studies with channeled heavy ions / D. Dauvergne ... [et al.]. Crystal assisted atomic physics experiments using heavy ions / K. Komaki -- Collisions involving clusters and surfaces. Structure and dynamics of Van der Waal complexes: from triatomic to medium size clusters / G. Delgado Barrio ... [et al.]. Evaporation, fission and multifragmentation processes of multicharged C[symbol] ions versus excitation energies / S. Martin ... [et al.]. Fragmentation of collisionally excited fullerenes / M. Alcami, S. Diaz-Tendero and F. Martín. Lifetimes of C[symbol] and C[symbol] dianions in a storage ring / S. Tomita ... [et al.]. Clusters and clusters of clusters in collisions / B. Manil ... [et al

  6. Electron-Atom Collisions in Gases

    ERIC Educational Resources Information Center

    Kraftmakher, Yaakov

    2013-01-01

    Electron-atom collisions in gases are an aspect of atomic physics. Three experiments in this field employing a thyratron are described: (i) the Ramsauer-Townsend effect, (ii) the excitation and ionization potentials of xenon and (iii) the ion-electron recombination after interrupting the electric discharge.

  7. Atomic physics

    SciTech Connect

    Livingston, A.E.; Kukla, K.; Cheng, S.

    1995-08-01

    In a collaboration with the Atomic Physics group at Argonne and the University of Toledo, the Atomic Physics group at the University of Notre Dame is measuring the fine structure transition energies in highly-charged lithium-like and helium-like ions using beam-foil spectroscopy. Precise measurements of 2s-2p transition energies in simple (few-electron) atomic systems provide stringent tests of several classes of current atomic- structure calculations. Analyses of measurements in helium-like Ar{sup 16+} have been completed, and the results submitted for publication. A current goal is to measure the 1s2s{sup 3}S{sub 1} - 1s2p{sup 3}P{sub 0} transition wavelength in helium-like Ni{sup 26+}. Measurements of the 1s2s{sup 2}S{sub 1/2} - 1s2p{sup 2}P{sub 1/2,3/2} transition wavelengths in lithium-like Kr{sup 33+} is planned. Wavelength and lifetime measurements in copper-like U{sup 63+} are also expected to be initiated. The group is also participating in measurements of forbidden transitions in helium-like ions. A measurement of the lifetime of the 1s2s{sup 3}S{sub 1} state in Kr{sup 34+} was published recently. In a collaboration including P. Mokler of GSI, Darmstadt, measurements have been made of the spectral distribution of the 2E1 decay continuum in helium-like Kr{sup 34+}. Initial results have been reported and further measurements are planned.

  8. Theory of slow atomic collisions

    NASA Astrophysics Data System (ADS)

    Nikitin, E. E.; Umanskii, S. Ia.

    The theory presented in this book is self-contained. It can be applied to the interpretation of various processes occurring in atomic collisions over a relatively wide energy range, from thermal energies to hundreds of eV. The general formulation of the scattering problem under quasi-classical conditions is discussed, taking into account scattering amplitudes and cross sections, scattering equations, collisions of two many-electron atoms, and integral cross sections for isotropic collisions. Other topics explored are related to diatomic electronic states, approximate calculations of the electronic states of diatoms, elastic scattering, approximate calculations of a multichannel quasi-classical scattering matrix, the two-state scattering problem, the linear two-state Landau-Zener model, nonlinear two-state models of nonadiabatic coupling, multistate models of nonadiabatic coupling, and a case study involving intramultiplet mixing and depolarization of alkalis in collisions with noble gases.

  9. Atom trap loss, elastic collisions, and technology

    NASA Astrophysics Data System (ADS)

    Booth, James

    2012-10-01

    The study of collisions and scattering has been one of the most productive approaches for modern physics, illuminating the fundamental structure of crystals, surfaces, atoms, and sub-atomic particles. In the field of cold atoms, this is no less true: studies of cold atom collisions were essential to the production of quantum degenerate matter, the formation of cold molecules, and so on. Over the past few years it has been my delight to investigate elastic collisions between cold atoms trapped in either a magneto-optical trap (MOT) or a magnetic trap with hot, background gas in the vacuum environment through the measurement of the loss of atoms from the trap. Motivated by the goal of creating cold atom-based technology, we are deciphering what the trapped atoms are communicating about their environment through the observed loss rate. These measurements have the advantages of being straightforward to implement and they provide information about the underlying, fundamental inter-atomic processes. In this talk I will present some of our recent work, including the observation of the trap depth dependence on loss rate for argon-rubidium collisions. The data follow the computed loss rate curve based on the long-range Van der Waals interaction between the two species. The implications of these findings are exciting: trap depths can be determined from the trap loss measurement under controlled background density conditions; observation of trap loss rate in comparison to models for elastic, inelastic, and chemical processes can lead to improved understanding and characterization of these fundamental interactions; finally the marriage of cold atoms with collision modeling offers the promise of creating a novel pressure sensor and pressure standard for the high and ultra-high vacuum regime.

  10. Photonic, Electronic and Atomic Collisions

    NASA Astrophysics Data System (ADS)

    Fainstein, Pablo D.; Lima, Marco Aurelio P.; Miraglia, Jorge E.; Montenegro, Eduardo C.; Rivarola, Roberto D.

    2006-11-01

    Plenary. Electron collisions - past, present and future / J. W. McConkey. Collisions of slow highly charged ions with surfaces / J. Burgdörfer ... [et al.]. Atomic collisions studied with "reaction-microscopes" / R. Moshammer ... [et al.]. Rydberg atoms: a microscale laboratory for studying electron-molecule tnteractions / F. B. Dunning -- Collisions involvintg photons. Quantum control of photochemical reaction dynamics and molecular functions / M. Yamaki ... [et al.]. Manipulating and viewing Rydberg wavepackets / R. R. Jones. Angle-resolved photoelectrons as a probe of strong-field interactions / M. Vrakking. Ultracold Rydberg atoms in a structured environment / I. C. H. Liu and J. M. Rost. Synchrotron-radiation-based recoil ion momentum spectroscopy of laser cooled and trapped cesium atoms / L. H. Coutinho. Reconstruction of attosecond pulse trains / Y. Mairesse ... [et al.]. Selective excitation of metastable atomic states by Femto- and attosecond laser pulses / A. D. Kondorskiy. Accurate calculations of triple differential cross sections for double photoionization of the hygrogen molecule / W. Vanroose ... [et al.]. Double and triple photoionization of Li and Be / J. Colgan, M. S. Pindzola and F. Robicheaux. Few/many body dynamics in strong laser fields / J. Zanghellini and T. Brabec. Rescattering-induced effects in electron-atom scattering in the presence of a circularly polarized laser field / A. V. Flegel ... [et al.]. Multidimensional photoelectron spectroscopy / P. Lablanquie ... [et al.]. Few photon and strongly driven transitions in the XUV and beyond / P. Lambropoulos, L. A. A. Nikolopoulos and S. I. Themelis. Ionization dynamics of atomic clusters in intense laser pulses / U. Saalmann and J. M. Rost. On the second order autocorrelation of an XUV attosecond pulse train / E. P. Benis ... [et al.]. Evidence for rescattering in molecular dissociation / I. D. Williams ... [et al.]. Photoionizing ions using synchrotron radiation / R. Phaneuf. Photo double

  11. Ion-Atom Cold Collisions and Atomic Clocks

    NASA Technical Reports Server (NTRS)

    Prestage, John D.; Maleki, Lute; Tjoelker, Robert L.

    1997-01-01

    Collisions between ultracold neutral atoms have for some time been the subject of investigation, initially with hydrogen and more recently with laser cooled alkali atoms. Advances in laser cooling and trapping of neutral atoms in a Magneto-Optic Trap (MOT) have made cold atoms available as the starting point for many laser cooled atomic physics investigations. The most spectacularly successful of these, the observation of Bose-Einstein Condensation (BEC) in a dilute ultra-cold spin polarized atomic vapor, has accelerated the study of cold collisions. Experimental and theoretical studies of BEC and the long range interaction between cold alkali atoms is at the boundary of atomic and low temperature physics. Such studies have been difficult and would not have been possible without the development and advancement of laser cooling and trapping of neutral atoms. By contrast, ion-atom interactions at low temperature, also very difficult to study prior to modern day laser cooling, have remained largely unexplored. But now, many laboratories worldwide have almost routine access to cold neutral atoms. The combined technologies of ion trapping, together with laser cooling of neutrals has made these studies experimentally feasible and several very important, novel applications might come out of such investigations . This paper is an investigation of ion-atom interactions in the cold and ultra-cold temperature regime. Some of the collisional ion-atom interactions present at room temperature are very much reduced in the low temperature regime. Reaction rates for charge transfer between unlike atoms, A + B(+) approaches A(+) + B, are expected to fall rapidly with temperature, approximately as T(sup 5/2). Thus, cold mixtures of atoms and ions are expected to coexist for very long times, unlike room temperature mixtures of the same ion-atom combination. Thus, it seems feasible to cool ions via collisions with laser cooled atoms. Many of the conventional collisional interactions

  12. The problems of solar-terrestrial coupling and new processes introduced to the physics of the ionosphere from the physics of atomic collisions

    NASA Astrophysics Data System (ADS)

    Avakyan, Sergei

    2010-05-01

    Further progress in research of solar-terrestrial coupling requires better understanding of solar variability influence on the ionosphere. The most powerful manifestations of solar variability are solar flares and geomagnetic storms. During a flare EUV/X-ray irradiations are completely absorbed in the ionosphere producing SID. During geomagnetic storms precipitations of electrons with energy of several keV (and to a lesser extent protons precipitations) from radiation belts and geomagnetosphere produce additional ionization and low latitude auroras. Considering the physics of ionosphere during the last several decades we have been taking into account three novel processes well known in the physics of atomic collisions. These are Auger effect [S. V. Avakyan, The consideration of Auger processes in the upper atmosphere of Earth. In Abstracts of paper presented at the Tenth scien. and techn. Conf. of young specialists of S.I. Vavilov State Optical Institute, 1974, 29-31.], multiple photoionization of upper, valence shell [S.V. Avakyan, The source of O++ ions in the upper atmosphere, 1979, Cosmic Res, 17, 942 - 943] and Rydberg excitation of all the components of upper atmosphere [S.V. Avakyan, The new factor in the physics of solar - terrestrial relations - Rydberg atomic and molecules states. Conf. on Physics of solar-terrestrial relationships, 1994, Almaty, 3 - 5]. In the present paper the results of bringing these new processes in the ionospheric physics are discussed and also its possible role in the physics of solar-terrestrial coupling is considered. Involving these processes to the model estimations allowed us for the first time to come to the following important conclusions: - Auger electrons play the determinant role at the formation of energy spectrum of photoelectrons and secondary auroral electrons at the range above 150 eV; - double photoionization of the outer shell of the oxygen atom (by a single photon) plays a dominant role in the formation of

  13. Atomic and Molecular Physics

    NASA Technical Reports Server (NTRS)

    Bhatia, Anand K.

    2005-01-01

    A symposium on atomic and molecular physics was held on November 18, 2005 at Goddard Space Flight Center. There were a number of talks through the day on various topics such as threshold law of ionization, scattering of electrons from atoms and molecules, muonic physics, positron physics, Rydberg states etc. The conference was attended by a number of physicists from all over the world.

  14. Advances in atomic physics

    PubMed Central

    El-Sherbini, Tharwat M.

    2013-01-01

    In this review article, important developments in the field of atomic physics are highlighted and linked to research works the author was involved in himself as a leader of the Cairo University – Atomic Physics Group. Starting from the late 1960s – when the author first engaged in research – an overview is provided of the milestones in the fascinating landscape of atomic physics. PMID:26425356

  15. Transition rates in proton - Rydberg atom collisions

    NASA Astrophysics Data System (ADS)

    Vrinceanu, Daniel

    2016-05-01

    Monte Carlo simulations for energy and angular momentum transfer processes in proton - Ryderg atom collisions were performed and the corresponding rates are reported.The relevance of these rates in the context of cosmological recombination is discussed. The rates are contrasted with the similar rates in electron - Rydberg atom collisions. This work has been supported by National Science Foundation through grants for the Center for Research on Complex Networks (HRD-1137732) and Research Infrastructure for Science and Engineering (RISE) (HRD-1345173).

  16. Multiple-electron processes in fast ion-atom collisions

    SciTech Connect

    Schlachter, A.S.

    1989-03-01

    Research in atomic physics at the Lawrence Berkeley Laboratory Super-HILAC and Bevalac accelerators on multiple-electron processes in fast ion-atom collisions is described. Experiments have studied various aspects of the charge-transfer, ionization, and excitation processes. Examples of processes in which electron correlation plays a role are resonant transfer and excitation and Auger-electron emission. Processes in which electron behavior can generally be described as uncorrelated include ionization and charge transfer in high-energy ion-atom collisions. A variety of experiments and results for energies from 1 MeV/u to 420 MeV/u are presented. 20 refs., 15 figs.

  17. Electron-atom /molecule/ collision processes

    NASA Technical Reports Server (NTRS)

    Trajmar, S.

    1980-01-01

    Electron-atom (molecule) collision processes at low and intermediate energies, from near threshold to a few hundred electron volts, are discussed. Attention is given to experimental techniques and procedures, electron impact cross sections, impact excitation and electron-atom scattering in laser fields. Specific examples are presented that illustrate various experimental techniques and interpretations of observations.

  18. Role of atomic collisions in fusion

    SciTech Connect

    Post, D.E.

    1982-04-01

    Atomic physics issues have played a large role in controlled fusion research. A general discussion of the present role of atomic processes in both magnetic and inertial controlled fusion work is presented.

  19. Positronium collisions with rare-gas atoms

    NASA Astrophysics Data System (ADS)

    Gribakin, G. F.; Swann, A. R.; Wilde, R. S.; Fabrikant, I. I.

    2016-03-01

    We calculate elastic scattering of positronium (Ps) by the Xe atom using the recently developed pseudopotential method (Fabrikant and Gribakin 2014 Phys. Rev. A 90 052717) and review general features of Ps scattering from heavier rare-gas atoms: Ar, Kr and Xe. The total scattering cross section is dominated by two contributions: elastic scattering and Ps ionization (break-up). To calculate the Ps ionization cross sections we use the binary-encounter method for Ps collisions with an atomic target. Our results for the ionization cross section agree well with previous calculations carried out in the impulse approximation. Our total Ps-Xe cross section, when plotted as a function of the projectile velocity, exhibits similarity with the electron-Xe cross section for the collision velocities higher than 0.8 a.u., and agrees very well with the measurements at Ps velocities above 0.5 a.u.

  20. Electron collisions with coherently prepared atomic targets

    SciTech Connect

    Trajmar, S.; Kanik, I.; LeClair, L.R.; Khakoo, M.S.; Bray, I.; Fursa, D.; Csanak, G.

    1998-02-01

    The subject of electron scattering by laser-excited atoms is briefly reviewed. To demonstrate some aspects of these electron collision processes, the authors describe the procedures and the results of a joint experimental and theoretical study concerning elastic scattering by coherently excited {sup 138}Ba (...6s6p {sup 1}P{sub 1}) atoms. Examples of experimental and theoretical collision parameters and magnetic sublevel differential cross sections for elastic scattering are given and compared. The convergent close coupling calculations (with the neglect of spin-orbit interaction) are in good agreement with experiment at 20 eV impact energy and 10, 15 and 20{degree} scattering angles and can be expected to yield reliable integral magnetic sublevel and alignment creation cross sections. The role of these quantities in plasma polarization spectroscopy is pointed out.

  1. Cold collisions of alkali-metal atoms and chromium atoms

    NASA Astrophysics Data System (ADS)

    Jeung, G.-H.; Hagebaum-Reignier, D.; Jamieson, M. J.

    2010-12-01

    We present ab initio potentials for ground state lithium, sodium, potassium and rubidium atoms interacting with ground state chromium atoms via the 6Σ+ and 8Σ+ states of the corresponding dimers. Each potential is matched to the leading van der Waals dispersion energy -C6/R6 - C8/R8 and an exchange energy; we list the values of C6, C8 and the exchange fitting parameters. We present calculated values from quantal and semi-classical approximations for the s-wave scattering length and effective range and the p-wave scattering volume for collisions of each of the alkali-metal atoms lithium, sodium, potassium and rubidium with 52chromium atoms and comment on s-wave scattering by 53chromium atoms.

  2. Atom-atom inelastic collisions and three-body atomic recombination in weakly ionized argon plasmas

    NASA Technical Reports Server (NTRS)

    Braun, C. G.; Kunc, J. A.

    1989-01-01

    A stationary collisional-radiative model including both inelastic electron-atom and atom-atom collisions is used to examine nonequilibrium weakly ionized argon plasmas with atomic densities 10 to the 16th to 10 to the 20th/cu cm, temperatures below 6000 K, and with different degrees of radiation trapping. It is shown that three-body atomic recombination becomes important at high particle densities. Comparison is made between the present approach and Thomson's theory for atomic recombination.

  3. Description of ionization in the molecular approach to atomic collisions

    SciTech Connect

    Harel, C.; Jouin, H.; Pons, B.; Errea, L.F.; Mendez, L.; Riera, A.

    1997-01-01

    Molecular treatments of atomic collisions have traditionally been restricted to low nuclear velocities because of their failure to reproduce the fall of the capture cross sections at higher velocities. The limitation has recently been seen to be due to their description of ionizing processes. This feature is shown here to be a general one for multicharged ion-atom collisions. Its origin and characteristics are described and illustrated for the prototypical Li{sup 3+}+H(1s) reaction. Ionization appears as a result of the inertia of the electron cloud to adiabatically follow the nuclear motion. This gives rise to nonadiabatic transitions, which represent an ionizing flux whenever the nuclear velocity is high enough that the energy of the traveling molecular orbitals involved is positive in both moving atomic reference frames. Two strongly connected mechanisms appear, corresponding to the relative translational and rotational nuclear motions. Because of the finiteness of the basis, these mechanisms terminate with unphysical trapping effects. While interesting {ital per se}, knowledge of these features is also useful with respect to improving molecular treatments of atomic collisions with the addition of pseudostates. {copyright} {ital 1996} {ital The American Physical Society}

  4. Atomic collision databases and data services -- A survey

    SciTech Connect

    Schultz, D.R.

    1997-12-31

    Atomic collision databases and data services constitute an important resource for scientific and engineering applications such as astrophysics, lighting, materials processing, and fusion energy, as well as an important knowledge base for current developments in atomic collision physics. Data centers and research groups provide these resources through a chain of efforts that include producing and collecting primary data, performing evaluation of the existing data, deducing scaling laws and semiempirical formulas to compactly describe and extend the data, producing the recommended sets of data, and providing convenient means of maintaining, updating, and disseminating the results of this process. The latest efforts have utilized modern database, storage, and distribution technologies including the Internet and World Wide Web. Given here is an informal survey of how these resources have developed, how they are currently characterized, and what their likely evolution will lead them to become in the future.

  5. Atomic collision databases and data services-a survey

    NASA Astrophysics Data System (ADS)

    Schultz, David R.

    1998-07-01

    Atomic collision databases and data services constitute an important resource for scientific and engineering applications such as astrophysics, lighting, materials processing, and fusion energy, as well as an important knowledge base for current developments in atomic collision physics. Data centers and research groups provide these resources through a chain of efforts that include producing and collecting primary data, performing evaluation of the existing data, deducing scaling laws and semiempirical formulas to compactly describe and extend the data, producing recommended sets of data, and providing convenient means of maintaining, updating, and disseminating the results of this process. The latest efforts have utilized modern database, storage, and distribution technologies including the Internet and World Wide Web. Given here is an informal survey of how these resources have developed, how they are currently characterized, and what their likely evolution will lead them to become in the future.

  6. Positronium collisions with rare-gas atoms

    NASA Astrophysics Data System (ADS)

    Fabrikant, Ilya; Gribakin, Gleb; Swann, Andrew; Wilde, Robyn

    2016-05-01

    We calculate elastic scattering of positronium (Ps) by the Xe atom using the recently developed pseudopotential method† and review general features of Ps scattering from heavier rare-gas atoms: Ar, Kr and Xe. The total scattering cross section is dominated by two contributions: elastic scattering and Ps ionization (break-up). To calculate the Ps ionization cross sections we use the binary-encounter method for Ps collisions with an atomic target. Our results for the ionization cross section agree well with previous calculations carried out in the impulse approximation. Our total Ps-Xe cross section, when plotted as a function of the projectile velocity, exhibits similarity with the electron-Xe cross section for the collision velocities higher than 0.8 a.u., and agrees very well with the measurements at Ps velocities above 0.5 a.u. † Fabrikant I I and Gribakin G F 2014 Phys. Rev. A 90 052717 Supported by the US National Science Foundation.

  7. Ionization Phenomena in Ion-Atom Collisions

    NASA Astrophysics Data System (ADS)

    Deveney, Edward Francis

    Two many-electron ion-atom collision systems are used to investigate atomic and molecular structure and collisional interactions. Electrons emitted from MeV/u C^{3+} projectile target -atom collisions were measured with a high-resolution position -sensitive electron spectrometer at Oak Ridge National Laboratory. The electrons are predominantly ionized by direct projectile -target interactions or autoionizing (AI) from doubly excited AI levels of the ion which were excited in the collision. The energy dependence of directly scattered target electrons, binary-encounter electrons (BEE), is investigated and compared with theory. AI levels of the projectile 1s to nl single electron excited series, (1s2snl) n = 2,3,4,....infty, including the series limit are identified uniquely using energy level calculations. Original Auger yield calculations using a code by Cowan were used to discover a 1/{n^3} scaling in intensities of Auger peaks in the aforementioned series. This is explained using scattering theory. A nonstatistical population of the terms in the (1s2s2l) configuration was identified and investigated as a function of the beam energy and for four different target atoms. Two electron excited configurations are identified and investigated. The angular distribution of a correlated transfer and excitation AI state is measured and compared to theory. The final scattered charge state distributions of Kr^ {n+}, n = 1, 2, 3, 4, 5, projectiles are measured following collisions with Kr targets in the Van de Graaff Laboratory here at The University of Connecticut. Average scattered charge states as high as 12 are observed. It appears that these electrons are ionized during the lifetime of the quasimolecular state but a complete picture of the ionization mechanism(s) is not known. Calculations using a statistical model of ionization, modified in several ways, are compared with the experimental results to see if it is possible to isolate whether or not the electrons originate

  8. Atomic physics with highly charged ions. Progress report

    SciTech Connect

    Richard, P.

    1994-08-01

    The study of inelastic collision phenomena with highly charged projectile ions and the interpretation of spectral features resulting from these collisions remain as the major focal points in the atomic physics research at the J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas. The title of the research project, ``Atomic Physics with Highly Charged Ions,`` speaks to these points. The experimental work in the past few years has divided into collisions at high velocity using the primary beams from the tandem and LINAC accelerators and collisions at low velocity using the CRYEBIS facility. Theoretical calculations have been performed to accurately describe inelastic scattering processes of the one-electron and many-electron type, and to accurately predict atomic transition energies and intensities for x rays and Auger electrons. Brief research summaries are given for the following: (1) electron production in ion-atom collisions; (2) role of electron-electron interactions in two-electron processes; (3) multi-electron processes; (4) collisions with excited, aligned, Rydberg targets; (5) ion-ion collisions; (6) ion-molecule collisions; (7) ion-atom collision theory; and (8) ion-surface interactions.

  9. Orientational rainbows in atom--molecule collisions

    SciTech Connect

    Vervaat, M.G.M.; Spalburg, M.R.; Los, J.; Kleyn, A.W.

    1984-11-01

    The experimental and calculated differential cross sections for ion pair formation in K (27 to 50 eV LAB) O/sub 2/ collisions show an orientational rainbow at small scattering angle. This rainbow is found to be due to the anisotropy of the K--O/sub 2/ interaction potential. Using the position of the orientational rainbow, the anisotropy in the repulsive part of the interaction potential is determined as G = (1+1.3( +- )*P/sub 2/(cos ..cap alpha..)), where P/sub 2/ is a Legendre polynomial and ..cap alpha.. the angle between the molecular axis and the radius vector of the atom. The interaction potential has the form V(R) = 102.9 exp(-0.571R)+(..delta..-1/R), where ..delta.. is the ionization potential of K minus the vertical electron affinity of O/sub 2/, the latter depending on the vibrational phase only; the term placed between the square brackets does not act during the complete collision, but only onward from that point during the collision where the ion-pair formation occurs.

  10. Correlated charge-changing ion-atom collisions

    SciTech Connect

    Tanis, J.A.

    1992-04-01

    This report summarizes the progress and accomplishments in accelerator atomic physics research supported by DOE grant DE-FG02-87ER13778 from March 16, 1991 through March 15, 1992. This work involves the experimental investigation of fundamental atomic processes in collisions of charged projectiles with neutral targets or electrons, with particular emphasis on two-electron interactions and electron correlation effects. Processes involving combinations of excitation, ionization, and charge transfer are investigated utilizing coincidence techniques in which projectiles charge-changing events are associated with x-ray emission, target recoil ions, or electron emission. New results have been obtained for studies involving (1) resonant recombination of atomic ions, (2) double ionization of helium, and (3) continuum electron emission. Experiments were conducted using accelerators at the Lawrence Berkeley Laboratory, Argonne National Laboratory, Michigan State University, Western Michigan University, and the Institute of Nuclear Research, Debrecen, Hungary. Brief summaries of work completed and work in progress are given in this report.

  11. Contemporary Aspects of Atomic Physics

    ERIC Educational Resources Information Center

    Knott, R. G. A.

    1972-01-01

    The approach generally used in writing undergraduate textbooks on Atomic and Nuclear Physics presents this branch as historical in nature. Describes the concepts of astrophysics, plasma physics and spectroscopy as contemporary and intriguing for modern scientists. (PS)

  12. Alignment and orientation in ion/endash/atom collisions

    SciTech Connect

    Kimura, M.; Lane, N.F.

    1987-01-01

    Recent progress in the theoretical study of alignment and orientation in atom-atom and ion-atom collisions at intermediate energies is reviewed. Recent systematic studies of the alignment and orientation of electronic charge cloud distributions of excited states resulting from such collisions clearly have provided more detailed information about the underlying collision dynamics. However, since accurate determination of these parameters is quite difficult, both theoretically and experimentally, a close collaboration between theory and experiment is necessary for a deeper understanding of the collision dynamics. A more complete approach, where the full density matrix is determined, is also discussed.

  13. Heavy particle atomic collisions in astrophysics: Beyond H and He targets

    SciTech Connect

    Stancil, P.C.; Krstic, P.S.; Schultz, D.R.

    1998-06-01

    The physical conditions relating to the emission of x-rays from Jovian and cometary atmospheres and to supernova ejecta are briefly described. Emphasis is placed on elucidating the relevance and importance of atomic collision processes, the availability of data, and the outstanding data needs for modeling these environments. Some preliminary theoretical studies of electron capture for important collisions systems, involving molecular and atomic metal targets, are presented.

  14. Many-Body Atomic Physics

    NASA Astrophysics Data System (ADS)

    Boyle, J. J.; Pindzola, M. S.

    2005-11-01

    Preface; Contributors; Introduction; Part I. Atomic Structure: 1. Development of atomic many-body theory Ingvar Lindgren; 2. Relativistic MBPT for highly charged ions W. R. Johnson; 3. Parity nonconservation in atoms S. A. Blundell, W. R. Johnson, and J. Sapirstein; Part II. Photoionization of Atoms: 4. Single photoionization processes J. J. Boyle, and M. D. Kutzner; 5. Photoionization dominated by double excitation T. N. Chang; 6. Direct double photoionization in atoms Z. W. Liu; 7. Photoelectron angular distributions Steven T. Manson; Part III. A. Atomic Scattering - General Considerations: 8. The many-body approach to electron-atom collisions M. Ya Amusia; 9. Theoretical aspects of electron impact ionization P. L. Altick; Part III. B. Atomic Scattering - Low-Order Applications: 10. Perturbation series methods D. H. Madison; 11. Target dependence of the triply differential cross section Cheng Pan and Anthony F. Starace; 12. Overview of Thomas processes for fast mass transfer J. H. McGuire, Jack C. Straton and T. Ishihara; Part III. C. Atomic Scattering - All-Order Applications: 13. R-matrix Theory: Some Recent Applications Philip G. Burke: 14. Electron scattering: application of Dirac R-matrix theory Wasantha Wijesundera, Ian Grant and Patrick Norrington; 15. Close coupling and distorted-wave theory D. C. Griffin and M. S. Pindzola; Appendix: Units and notation; References; Index.

  15. Many-Body Atomic Physics

    NASA Astrophysics Data System (ADS)

    Boyle, J. J.; Pindzola, M. S.

    1998-09-01

    Preface; Contributors; Introduction; Part I. Atomic Structure: 1. Development of atomic many-body theory Ingvar Lindgren; 2. Relativistic MBPT for highly charged ions W. R. Johnson; 3. Parity nonconservation in atoms S. A. Blundell, W. R. Johnson, and J. Sapirstein; Part II. Photoionization of Atoms: 4. Single photoionization processes J. J. Boyle, and M. D. Kutzner; 5. Photoionization dominated by double excitation T. N. Chang; 6. Direct double photoionization in atoms Z. W. Liu; 7. Photoelectron angular distributions Steven T. Manson; Part III. A. Atomic Scattering - General Considerations: 8. The many-body approach to electron-atom collisions M. Ya Amusia; 9. Theoretical aspects of electron impact ionization P. L. Altick; Part III. B. Atomic Scattering - Low-Order Applications: 10. Perturbation series methods D. H. Madison; 11. Target dependence of the triply differential cross section Cheng Pan and Anthony F. Starace; 12. Overview of Thomas processes for fast mass transfer J. H. McGuire, Jack C. Straton and T. Ishihara; Part III. C. Atomic Scattering - All-Order Applications: 13. R-matrix Theory: Some Recent Applications Philip G. Burke: 14. Electron scattering: application of Dirac R-matrix theory Wasantha Wijesundera, Ian Grant and Patrick Norrington; 15. Close coupling and distorted-wave theory D. C. Griffin and M. S. Pindzola; Appendix: Units and notation; References; Index.

  16. Applications of atomic and molecular data to radiation physics

    SciTech Connect

    Inokuti, M.

    1982-01-01

    The general purpose of our work is to provide atomic and molecular collision cross sections useful for radiological physics, dosimetry, and other applications. Studies on the systematics of atomic oscillator-strength spectra and a survey of stopping power data are briefly described. (WHK)

  17. Experimental atomic physics in heavy-ion storage rings

    SciTech Connect

    Datz, S.; Andersen, L.H.; Briand, J.P.; Liesen, D.

    1987-01-01

    This paper outlines the discussion which took place at the ''round table'' on experimental atomic physics in heavy-ion storage rings. Areas of discussion are: electron-ion interactions, ion-ion collisions, precision spectroscopy of highly charged ions, beta decay into bound final states, and atomic binding energies from spectroscopy of conversion elections. 18 refs., 1 tab. (LSP)

  18. Landau quantization effects in ultracold atom-ion collisions

    NASA Astrophysics Data System (ADS)

    Simoni, Andrea; Launay, Jean-Michel

    2011-12-01

    We study ultracold atom-ion collisions in the presence of an external magnetic field. At low collision energy the field can drastically modify the translational motion of the ion, which follows quantized cyclotron orbits. We present a rigorous theoretical approach for the calculation of quantum scattering amplitudes in these conditions. Collisions in different magnetic field regimes, identified by the size of the cyclotron radius with respect to the range of the interaction potential, are investigated. Our results are important in cases where use of a magnetic field to control the atom-ion collision dynamics is envisioned.

  19. Overview on collision processes of highly charged ions with atoms present status and problems

    SciTech Connect

    Janev, R.K.

    1983-05-01

    This paper provides a brief discussion on the present status of the collision physics of highly charged ions with atoms. The emphasis is on the main achievements in understanding and describing the most important collision processes, and as charge transfer, ionization and Auger-type processes, and even more on those open problems which, due either to their scientific or practical importance, represent challenges to current research in this field. The paper concentrates on general ideas and problems whose development and solutions have advanced or will advance our basic understanding of the collision dynamics of multiply charged ions with atoms.

  20. Ultracold collisions between Rb atoms and a Sr+ ion

    NASA Astrophysics Data System (ADS)

    Meir, Ziv; Sikorsky, Tomas; Ben-Shlomi, Ruti; Dallal, Yehonatan; Ozeri, Roee

    2015-05-01

    In last decade, a novel field emerged, in which ultracold atoms and ions in overlapping traps are brought into interaction. In contrast to the short ranged atom-atom interaction which scales as r-6, atom-ion potential persists for hundreds of μm's due to its lower power-law scaling - r-4. Inelastic collisions between the consistuents lead to spin and charge transfer and also to molecule formation. Elastic collisions control the energy transfer between the ion and the atoms. The study of collisions at the μK range has thus far been impeded by the effect of the ion's micromotion which limited collision energy to mK scale. Unraveling this limit will allow to investigate few partial wave and even S-wave collisions. Our system is capable of trapping Sr+ ions and Rb and Sr atoms and cooling them to their quantum ground state. Atoms and ions are trapped and cooled in separate chambers. Then, the atoms are transported using an optical conveyer belt to overlap the ions. In contrast to other experiments in this field where the atoms are used to sympathetic cool the ion, our system is also capable of ground state cooling the ion before immersing it into the atom cloud. By this method, we would be able to explore heating and cooling dynamics in the ultracold regime.

  1. Four Weeks of Atomic Physics.

    ERIC Educational Resources Information Center

    Lo Presto, Michael C.

    1995-01-01

    Describes a strategy for presenting ideas of atomic physics in the laboratory portion of the course before it is introduced during a lecture in order to give students an appreciation for the concepts involved, a historical look at how the field developed, and a comprehensive review of physics concepts. Presents a worksheet for the Bohr atom…

  2. Collision assisted Zeeman cooling with multiple types of atoms

    NASA Astrophysics Data System (ADS)

    Hamilton, Mathew S.; Wilson, Rebekah F.; Roberts, Jacob L.

    2014-01-01

    Through a combination of spin-exchange collisions in a magnetic field and optical pumping, it is possible to cool a gas of atoms without requiring the loss of atoms from the gas. This technique, collision assisted Zeeman cooling (CAZ), was developed theoretically assuming a single atomic species [G. Ferrari, Eur. Phys. J. D 13, 67 (2001)]. We have extended this cooling technique to a system of two atomic species rather than just one and have developed a simple analytic model describing the cooling rate. We find that the two-isotope CAZ cooling scheme has a clear theoretical advantage in systems that are reabsorption limited.

  3. Positron collisions with alkali-metal atoms

    NASA Technical Reports Server (NTRS)

    Gien, T. T.

    1990-01-01

    The total cross sections for positron and electron collisions with potassium, sodium, lithium and rubidium are calculated, employing the modified Glauber approximation. The Modified Glauber cross sections for positron collision with potassium and sodium at low intermediate energies are found to agree reasonably well with existing experimental data.

  4. Effects of hydrogen atom spin exchange collisions on atomic hydrogen maser oscillation frequency

    NASA Technical Reports Server (NTRS)

    Crampton, S. B.

    1979-01-01

    Frequency shifts due to collisions between hydrogen atoms in an atomic hydrogen maser frequency standard are studied. Investigations of frequency shifts proportional to the spin exchange frequency shift cross section and those proportional to the duration of exchange collisions are discussed. The feasibility of operating a hydrogen frequency standard at liquid helium temperatures is examined.

  5. Inelastic transitions in slow heavy-particle atomic collisions

    SciTech Connect

    Krstic, P. S.; Reinhold, C. O.; Burgdo''rfer, J.

    2001-05-01

    It is a generally held belief that inelastic transition probabilities and cross sections in slow, nearly adiabatic atomic collisions decrease exponentially with the inverse of the collision velocity v [i.e., {sigma}{proportional_to}exp(-const/v)]. This notion is supported by the Landau-Zener approximation and the hidden crossings approximation. We revisit the adiabatic limit of ion-atom collisions and show that for very slow collisions radial transitions are dominated by the topology of the branch points of the radial velocity rather than the branch points of the energy eigensurface. This can lead to a dominant power-law dependence of inelastic cross sections, {sigma}{proportional_to}v{sup n}. We illustrate the interplay between different contributions to the transition probabilities in a one-dimensional collision system for which the exact probabilities can be obtained from a direct numerical solution of the time-dependent Scho''dinger equation.

  6. Newly appreciated roles for electrons in ion-atom collisions

    SciTech Connect

    Sellin, I.A. . Dept. of Physics and Astronomy Oak Ridge National Lab., TN )

    1990-01-01

    Since the previous Debrecen workshop on High-Energy Ion-Atom Collisions there have been numerous experiments and substantial theoretical developments in the fields of fast ion-atom and ion- solid collisions concerned with explicating the previously largely underappreciated role of electrons as ionizing and exciting agents in such collisions. Examples to be discussed include the double electron ionization problem in He; transfer ionization by protons in He; double excitation in He; backward scattering of electrons in He; the role of electron-electron interaction in determining beta parameters for ELC; projectile K ionization by target electrons; electron spin exchange in transfer excitation; electron impact ionization in crystal channels; resonant coherent excitation in crystal channels; excitation and dielectronic recombination in crystal channels; resonant transfer and excitation; the similarity of recoil ion spectra observed in coincidence with electron capture vs. electron loss; and new research on ion-atom collisions at relativistic energies.

  7. Treatment of ion-atom collisions using a partial-wave expansion of the projectile wavefunction

    SciTech Connect

    Foster, M; Colgan, J; Wong, T G; Madison, D H

    2008-01-01

    We present calculations of ion-atom collisions using a partial-wave expansion of the projectile wavefunction. Most calculations of ion-atom collisions have typically used classical or plane-wave approximations for the projectile wavefunction, since partial-wave expansions are expected to require prohibitively large numbers of terms to converge scattering quantities. Here we show that such calculations are possible using modern high-performance computing. We demonstrate the utility of our method by examining elastic scattering of protons by hydrogen and helium atoms, problems familiar to undergraduate students of atomic scattering. Application to ionization of helium using partial-wave expansions of the projectile wavefunction, which has long been desirable in heavy-ion collision physics, is thus quite feasible.

  8. Atomic Collisions and free Lepton Pair Production

    SciTech Connect

    Gueclue, M.C.; Yilmaz, M.

    2005-10-26

    In this work, we have calculated the total cross sections of electron-positron pair production for the collisions of fully stripped gold ions for various energies. We have also compared our calculation with other methods.

  9. Foreword: Collision and reaction cell techniques in atomic mass spectrometry

    SciTech Connect

    Koppenaal, David W.; Eiden, Greg C.

    2004-01-01

    This contribution is a guest editorial statement and technical assessment for a special issue of the Royal Society of Chemistry journal entitled Journal of Analytical Atomic Spectrometry (JAAS). The editorial introduces the subject area of collision and reaction cells in atomic mass spectrometry, reviews current literature and commercial instrumentation trends, and previews four perspective and numerous research articles contained in the special journal issue.

  10. Frequency evolution of radiatively assisted collisions of K Rydberg atoms

    SciTech Connect

    Renn, M.J.; Thomson, D.S.; Gallagher, T.F. )

    1994-01-01

    Ramsey interference fringes are observed in the line shape of resonant Rydberg-atom--Rydberg-atom collisions occurring in the presence of a radiation field of frequency comparable to the inverse of the collision time. At low frequencies the fringes are phase dependent, but at high frequencies they are not. We present a theoretical interpretation based on a quasistatic field description which connects the low- and high-frequency regimes. In the high-frequency regime, this model gives results equivalent to those obtained using a dressed-atom'' approach.

  11. Physics of Ultra-Peripheral Nuclear Collisions

    SciTech Connect

    Bertulani, Carlos A.; Klein, Spencer R.; Nystrand, Joakim

    2005-02-02

    Moving highly-charged ions carry strong electromagnetic fields which act as a field of photons. In collisions at large impact parameters, hadronic interactions are not possible, and the ions interact through photon-ion and photon-photon collisions known as ultra-peripheral collisions (UPC). Hadron colliders like the Relativistic Heavy Ion Collider (RHIC), the Tevatron and the Large Hadron Collider (LHC) produce photonuclear and two-photon interactions at luminosities and energies beyond that accessible elsewhere; the LHC will reach a {gamma}p energy ten times that of the Hadron-Electron Ring Accelerator (HERA). Reactions as diverse as the production of anti-hydrogen, photoproduction of the {rho}{sup 0}, transmutation of lead into bismuth and excitation of collective nuclear resonances have already been studied. At the LHC, UPCs can study many types of ''new physics''.

  12. Atomic and Molecular Collisions at Liquid Surfaces.

    PubMed

    Tesa-Serrate, Maria A; Smoll, Eric J; Minton, Timothy K; McKendrick, Kenneth G

    2016-05-27

    The gas-liquid interface remains one of the least explored, but nevertheless most practically important, environments in which molecular collisions take place. These molecular-level processes underlie many bulk phenomena of fundamental and applied interest, spanning evaporation, respiration, multiphase catalysis, and atmospheric chemistry. We review here the research that has, during the past decade or so, been unraveling the molecular-level mechanisms of inelastic and reactive collisions at the gas-liquid interface. Armed with the knowledge that such collisions with the outer layers of the interfacial region can be unambiguously distinguished, we show that the scattering of gas-phase projectiles is a promising new tool for the interrogation of liquid surfaces with extreme surface sensitivity. Especially for reactive scattering, this method also offers absolute chemical selectivity for the groups that react to produce a specific observed product. PMID:27090845

  13. Atomic and Molecular Collisions at Liquid Surfaces

    NASA Astrophysics Data System (ADS)

    Tesa-Serrate, Maria A.; Smoll, Eric J.; Minton, Timothy K.; McKendrick, Kenneth G.

    2016-05-01

    The gas-liquid interface remains one of the least explored, but nevertheless most practically important, environments in which molecular collisions take place. These molecular-level processes underlie many bulk phenomena of fundamental and applied interest, spanning evaporation, respiration, multiphase catalysis, and atmospheric chemistry. We review here the research that has, during the past decade or so, been unraveling the molecular-level mechanisms of inelastic and reactive collisions at the gas-liquid interface. Armed with the knowledge that such collisions with the outer layers of the interfacial region can be unambiguously distinguished, we show that the scattering of gas-phase projectiles is a promising new tool for the interrogation of liquid surfaces with extreme surface sensitivity. Especially for reactive scattering, this method also offers absolute chemical selectivity for the groups that react to produce a specific observed product.

  14. Collision dynamics of two 238U atomic nuclei.

    PubMed

    Golabek, Cédric; Simenel, Cédric

    2009-07-24

    Collisions of actinide nuclei form, during very short times of few 10;{-21} s, the heaviest ensembles of interacting nucleons available on Earth. Such collisions have been proposed as an alternative way to produce heavy and superheavy elements. They are also used to produce superstrong electric fields by the huge number of interacting protons to test spontaneous positron-electron (e;{+}e;{-}) pair emission predicted by the quantum electrodynamics theory. The time-dependent Hartree-Fock theory is used to study collision dynamics of two 238U atomic nuclei. In particular, the role of nuclear deformation on collision time and on reaction mechanisms such as nucleon transfer is emphasized. The highest collision times (approximately 4 x 10;{-21} s at 1200 MeV) should allow experimental signature of spontaneous e;{+}e;{-} emission in case of bare uranium ions. Surprisingly, we also observe ternary fission due to purely dynamical effects. PMID:19659346

  15. Collision Dynamics of Two {sup 238}U Atomic Nuclei

    SciTech Connect

    Golabek, Cedric; Simenel, Cedric

    2009-07-24

    Collisions of actinide nuclei form, during very short times of few 10{sup -21} s, the heaviest ensembles of interacting nucleons available on Earth. Such collisions have been proposed as an alternative way to produce heavy and superheavy elements. They are also used to produce superstrong electric fields by the huge number of interacting protons to test spontaneous positron-electron (e{sup +}e{sup -}) pair emission predicted by the quantum electrodynamics theory. The time-dependent Hartree-Fock theory is used to study collision dynamics of two {sup 238}U atomic nuclei. In particular, the role of nuclear deformation on collision time and on reaction mechanisms such as nucleon transfer is emphasized. The highest collision times (approx4x10{sup -21} s at 1200 MeV) should allow experimental signature of spontaneous e{sup +}e{sup -} emission in case of bare uranium ions. Surprisingly, we also observe ternary fission due to purely dynamical effects.

  16. Homonuclear ionizing collisions of laser-cooled metastable helium atoms

    SciTech Connect

    Stas, R. J. W.; McNamara, J. M.; Hogervorst, W.; Vassen, W.

    2006-03-15

    We present a theoretical and experimental investigation of homonuclear ionizing collisions of laser-cooled metastable (2 {sup 3}S{sub 1}) helium atoms, considering both the fermionic {sup 3}He and bosonic {sup 4}He isotopes. The theoretical description combines quantum threshold behavior, Wigner's spin-conservation rule, and quantum-statistical symmetry requirements in a single-channel model, complementing a more complete close-coupling theory that has been reported for collisions of metastable {sup 4}He atoms. The model is supported with measurements (in the absence of light fields) of ionization rates in magneto-optically trapped samples that contain about 3x10{sup 8} atoms of a single isotope. The ionization rates are determined from measurements of trap loss due to light-assisted collisions combined with comparative measurements of the ion production rate in the absence and presence of trapping light. Theory and experiment show good agreement.

  17. Graphical R-matrix atomic collision environment (G RACE): the problem specification stage

    NASA Astrophysics Data System (ADS)

    Scott, N. S.; McMinn, A.; Burke, P. G.; Burke, V. M.; Noble, C. J.

    1993-12-01

    In this paper we introduce the concept of a graphical R-matrix atomic collision environment (G RACE). G RACE couples the graphical capability of powerful workstations with the processing power of supercomputers to provide an environment for the study of atomic collision properties and processes. At the core of G RACE is a new generation R-matrix program package, which is used to compute properties characterising electron atom and electron ion collisions. One of the motivations behind the project is to render this package simple to use by novice and experienced users alike, thereby significantly improving its usefulness to the physics community. G RACE is composed of a problem specification stage, a computation stage, and an interpretation stage. The focus of this paper is a description of the X Window graphical user interface which constitutes the problem specification stage of G RACE.

  18. Optically pumped atoms with velocity- and spin-changing collisions at low gas pressures

    SciTech Connect

    Morgan, Steven W.; Happer, William

    2010-04-15

    We discuss optical pumping when (a) the collision rates of optically pumped atoms with atoms or molecules of the background gas are small enough that individual velocity groups can be preferentially excited by a monochromatic light beam, (b) the collision rates are still fast enough to partially transfer the spin polarization to other velocity groups, and (c) there are nonnegligible losses of polarization due to collisional spin relaxation and Larmor precession. These conditions lead to a strong correlation between the velocity and the spin polarization of the atoms - that is, to 'spin-tagging' of the different velocity groups. This regime is similar to that of optically pumped {sup 23}Na atoms of the Earth's upper atmosphere, but it is seldom encountered in laboratory experiments. For cooling and trapping experiments, the collision rates with background gas are negligible. For gas-cell experiments the velocity-changing rates are normally so fast compared to spin relaxation or Larmor precession rates that the atoms have a Maxwellian velocity distribution with negligible correlation between the spin polarization and the velocity. We analyze the limiting cases of strong and weak collisions, which change the velocity by a large or small fraction, respectively, of the mean thermal velocity. The Keilson-Storer model [J. Keilson and A. E. Storer, Q. Appl. Math. 10, 243 (1952)] is used to discuss strong collisions, with memory parameter {alpha}=0 and weak collisions with {alpha}{yields}1. For weak collisions, the physics can be modeled by coupled Fokker-Planck equations, identical to those for forced diffusion in a harmonic-oscillator potential well. In this limit there are solutions analogous to the quantum mechanical coherent states of a harmonic oscillator.

  19. Optically Pumped Atoms with Velocity- and Spin-Changing Collisions at Low Gas Pressures

    NASA Astrophysics Data System (ADS)

    Happer, William

    2010-03-01

    We discuss optical pumping when: (a) the collision rates of optically pumped atoms with atoms or molecules of the background gas are small enough that individual velocity groups can be preferentially excited by a monochromatic light beam, (b) the collision rates are still fast enough to partially transfer the spin polarization to other velocity groups, and (c) there are non-negligible losses of polarization due to collisional spin relaxation and Larmor precession. These conditions lead to a strong correlation between the velocity and the spin polarization of the atoms-that is, to ``spin-tagging'' of the different velocity groups. This regime is similar to that of optically pumped 23Na atoms of the earth's upper atmosphere, but it is seldom encountered in laboratory experiments. For cooling and trapping experiments, the collision rates with background gas are negligible. For gas-cell experiments the velocity-changing rates are normally so fast compared to spin relaxation or Larmor precession rates, that the atoms have a Maxwellian velocity distribution with negligible correlation between the spin-polarization and the velocity. We analyze the limiting cases of strong and weak collisions, which change the velocity by a large or small fraction, respectively, of the mean thermal velocity. The Keilson-Storer model (J. Keilson and A. E. Storer, Q. Appl. Math. 10, 243 (1952)) is used to discuss strong collisions, with memory parameter =0, and weak collisions with $-> 1. For weak collisions, the physics can be modelled by coupled Fokker-Planck equations, identical to those for forced diffusion in a harmonic-oscillator potential well. In this limit there are solutions analogous to the quantum-mechanical coherent states of a harmonic oscillator.

  20. Collisions of Electrons with Atomic Oxygen: Current Status

    NASA Technical Reports Server (NTRS)

    Johnson, P. V.; Kanik, I.; Tayal, S. S.

    2005-01-01

    In 1990, two significant reviews of electron-atomic-oxygen collision processes were published. Since that time, a large volume of both experimental and theoretical research into these processes has occurred. These data are reviewed and recommendations regarding existing data sets and future research in this area are made. Attention is given to the challenges associated with handling atomic oxygen in terms of both experiment and theory.

  1. Light assisted collisions in ultra cold Tm atom

    NASA Astrophysics Data System (ADS)

    Akimov, Alexey; Cojocaru, Ivan; Pyatchenkov, Sergey; Snigirev, Stepan; Luchnokov, Ilia; Sukachev, Denis; Kalganova, Elena; Sorokin, Vadim

    2016-05-01

    Recently laser cooled rare earth elements attracted considerable attention due to the high orbital and magnetic moments. Such a systems allow low-field Feshabach resonances enabling tunable in wide range interactions. In particular, thulium atom has one hole in 4f shell therefore having orbital moment of 3 in the ground state, magnetic moment of 4 Bohr magnetons in ground state. While magnetic moment of the thulium atom is less than that of Erbium or Dysprosium simpler level structure, possibility to capture thulium atoms and the dipole trap at 532 nm make thulium atom an extremely attractive subject for quantum simulations. Nevertheless collisional properties of thulium atom are not yet explored in details, in particular light assisted collision of thulium atom were not yet investigated. In this contribution, we performed studies of light assisted collisions near in Magneto optical trap operating on narrow 530.7 nm transition. We found, that light assisted inelastic binary collisions losses rate is around β ~10-9cm3cm3s s . Possible mechanism of losses from the trap are discussed

  2. PREFACE: XXVIth International Conference on Photonic, Electronic and Atomic Collisions

    NASA Astrophysics Data System (ADS)

    Orel, Ann; Starace, Anthony F.; Nikolić, Dragan; Berrah, Nora; Gorczyca, Thomas W.; Kamber, Emanuel Y.; Tanis, John A.

    2009-12-01

    The XXVIth International Conference on Photonic, Electronic and Atomic Collisions was held on the campus of Western Michigan University (WMU) in Kalamazoo during 22-28 July 2009. Kalamazoo, the home of a major state university amid pleasant surroundings, was a delightful place for the conference. The 473 scientific participants, 111 of whom were students, had many fruitful discussions and exchanges that contributed to the success of the conference. Participants from 43 countries made the conference truly international in scope. The 590 abstracts that were presented on the first four days formed the heart of the conference and provided ample opportunity for discussion. This change, allowing the conference to end with invited talks, was a departure from the format used at previous ICPEAC gatherings in which the conferences ended with a poster session. The abstracts were split almost equally between the three main conference areas, i.e., photonic, electronic, and atomic collisions, and the posters were distributed across the days of the conference so that approximately equal numbers of abstracts in the different areas were scheduled for each day. Of the total number of presented abstracts, 517 of these are included in this proceedings volume, the first time that abstracts have been published by ICPEAC. There were 5 plenary lectures covering the different areas of the conference: Paul Corkum (University of Ottawa) talked on attosecond physics with atoms and molecules, Serge Haroche (Collège de France) on non-destructive photon counting, Toshiyuki Azuma (Tokyo Metropolitan University) on resonant coherent excitation of highly-charged ions in crystals, Eva Lindroth (Stockholm University) on atomic structure effects, and Alfred Müller (Justus Liebig University) on resonance phenomena in electron- and photon-ion collisions. Two speakers gave very illuminating public lectures that drew many people from the local area, as well as conference participants: Patricia Dehmer

  3. Spin-axis relaxation in spin-exchange collisions of alkali-metal atoms

    NASA Astrophysics Data System (ADS)

    Kadlecek, S.; Walker, T.; Walter, D. K.; Erickson, C.; Happer, W.

    2001-05-01

    We present calculations of spin-relaxation rates of alkali-metal atoms due to the spin-axis interaction acting in binary collisions between the atoms. We show that for the high-temperature conditions of interest here, the spin-relaxation rates calculated with classical-path trajectories are nearly the same as those calculated with the distorted-wave Born approximation. We compare these calculations to recent experiments that used magnetic decoupling to isolate spin relaxation due to binary collisions from that due to the formation of triplet van der Waals molecules. The values of the spin-axis coupling coefficients deduced from measurements of binary collision rates are consistent with those deduced from molecular decoupling experiments, and follow a physically plausible scaling law for the spin-axis coupling coefficients.

  4. Optically pumped atoms with velocity- and spin-changing collisions at low gas pressures

    NASA Astrophysics Data System (ADS)

    Morgan, Steven W.; Happer, William

    2010-04-01

    We discuss optical pumping when (a) the collision rates of optically pumped atoms with atoms or molecules of the background gas are small enough that individual velocity groups can be preferentially excited by a monochromatic light beam, (b) the collision rates are still fast enough to partially transfer the spin polarization to other velocity groups, and (c) there are nonnegligible losses of polarization due to collisional spin relaxation and Larmor precession. These conditions lead to a strong correlation between the velocity and the spin polarization of the atoms—that is, to “spin-tagging” of the different velocity groups. This regime is similar to that of optically pumped Na23 atoms of the Earth’s upper atmosphere, but it is seldom encountered in laboratory experiments. For cooling and trapping experiments, the collision rates with background gas are negligible. For gas-cell experiments the velocity-changing rates are normally so fast compared to spin relaxation or Larmor precession rates that the atoms have a Maxwellian velocity distribution with negligible correlation between the spin polarization and the velocity. We analyze the limiting cases of strong and weak collisions, which change the velocity by a large or small fraction, respectively, of the mean thermal velocity. The Keilson-Storer model [J. Keilson and A. E. Storer, Q. Appl. Math. 10, 243 (1952)] is used to discuss strong collisions, with memory parameter α=0 and weak collisions with α→1. For weak collisions, the physics can be modeled by coupled Fokker-Planck equations, identical to those for forced diffusion in a harmonic-oscillator potential well. In this limit there are solutions analogous to the quantum mechanical coherent states of a harmonic oscillator.

  5. Scattering of cold-atom coherences by hot atoms: frequency shifts from background-gas collisions.

    PubMed

    Gibble, Kurt

    2013-05-01

    Frequency shifts from background-gas collisions currently contribute significantly to the inaccuracy of atomic clocks. Because nearly all collisions with room-temperature background gases that transfer momentum eject the cold atoms from the clock, the interference between the scattered and unscattered waves in the forward direction dominates these frequency shifts. We show they are ≈ 10 times smaller than in room-temperature clocks and that van der Waals interactions produce the cold-atom background-gas shift. General considerations allow the loss of the Ramsey fringe amplitude to bound this frequency shift. PMID:23683186

  6. Physics of Nuclear Collisions at High Energy

    SciTech Connect

    Hwa, Rudolph C.

    2012-05-01

    A wide range of problems has been investigated in the research program during the period of this grant. Although the major effort has been in the subject of heavy-ion collisions, we have also studied problems in biological and other physical systems. The method of analysis used in reducing complex data in multiparticle production to simple descriptions can also be applied to the study of complex systems of very different nature. Phase transition is an important phenomenon in many areas of physics, and for heavy-ion collisions we study the fluctuations of multiplicities at the critical point. Human brain activities as revealed in EEG also involve fluctuations in time series, and we have found that our experience enables us to find the appropriate quantification of the fluctuations in ways that can differentiate stroke and normal subjects. The main topic that characterizes the research at Oregon in heavy-ion collisions is the recombination model for the treatment of the hadronization process. We have avoided the hydrodynamical model partly because there is already a large community engaged in it, but more significantly we have found the assumption of rapid thermalization unconvincing. Recent results in studying LHC physics lead us to provide more evidence that shower partons are very important even at low p_T, but are ignored by hydro. It is not easy to work in an environment where the conventional wisdom regards our approach as being incorrect because it does not adhere to the standard paradigm. But that is just what a vibrant research community needs: unconventional approach may find evidences that can challenge the orthodoxy. An example is the usual belief that elliptic flow in fluid dynamics gives rise to azimuthal anisotropy. We claim that it is only sufficient but not necessary. With more data from LHC and more independent thinkers working on the subject what is sufficient as a theory may turn out to be incorrect in reality. Another area of investigation that

  7. Few electron transitions in atomic collisions. Final report, September 1, 1992--December 31, 1995

    SciTech Connect

    McGuire, J.

    1997-04-01

    During the past three years we have evaluated probabilities and cross sections for few and multiple electron transitions in atomic collisions. Our studies included interactions of atoms and molecules with incident protons, bare ions, electrons, positrons, anti-protons, ions carrying electrons and photons. We also: studied the inter-relation between collisions with charged particles and collisions involving various processes with photons. This work has complemented various studies of collisions of atoms with charged particles and with photons as well as more general efforts to understand the nature of multi-electron systems. Our aim has been to begin with relatively simple two electron systems and to focus on fast processes in which there is too little time for complicated processes to occur. We have used a variety of computational techniques, but we emphasize those appropriate for fast collisions in which we hope to obtain insight into the physical nature of the process itself. We generally considered systems in which experimental data was available.

  8. Atomic Physics with Accelerators: Projectile Electron Spectroscopy (APAPES)

    NASA Astrophysics Data System (ADS)

    Madesis, I.; Dimitriou, A.; Laoutaris, A.; Lagoyannis, A.; Axiotis, M.; Mertzimekis, T.; Andrianis, M.; Harissopulos, S.; Benis, E. P.; Sulik, B.; Valastyán, I.; Zouros, T. J. M.

    2015-01-01

    The new research initiative APAPES (http://apapes.physics.uoc.gr/) has already established a new experimental station with a beam line dedicated for atomic collisions physics research, at the 5 MV TANDEM accelerator of the National Research Centre "Demokritos" in Athens, Greece. A complete zero-degree Auger projectile spectroscopy (ZAPS) apparatus has been put together to perform high resolution studies of electrons emitted in ion-atom collisions. A single stage hemispherical spectrometer with a 2-dimensional Position Sensitive Detector (PSD) combined with a doubly-differentially pumped gas target will be used to perform a systematic isoelectronic investigation of K-Auger spectra emitted from collisions of preexcited and ground state He-like ions with gas targets using novel techniques. Our intention is to provide a more thorough understanding of cascade feeding of the 1s2s2p 4P metastable states produced by electron capture in collisions of He-like ions with gas targets and further elucidate their role in the non-statistical production of excited three-electron 1s2s2p states by electron capture, recently a field of conflicting interpretations awaiting further resolution. At the moment, the apparatus is being completed and the spectrometer will soon be fully operational. Here we present the project progress and the recent high resolution spectrum obtained in collisions of 12 MeV C4+ on a Neon gas target.

  9. Coherent coupling of alkali atoms by random collisions.

    PubMed

    Katz, Or; Peleg, Or; Firstenberg, Ofer

    2015-09-11

    Random spin-exchange collisions in warm alkali vapor cause rapid decoherence and act to equilibrate the spin state of the atoms in the vapor. In contrast, here we demonstrate experimentally and theoretically a coherent coupling of one alkali species to another species, mediated by these random collisions. We show that the minor species (potassium) inherits the magnetic properties of the dominant species (rubidium), including its lifetime (T_{1}), coherence time (T_{2}), gyromagnetic ratio, and spin-exchange relaxation-free magnetic-field threshold. We further show that this coupling can be completely controlled by varying the strength of the magnetic field. Finally, we explain these phenomena analytically by mode mixing of the two species via spin-exchange collisions. PMID:26406827

  10. Bringing Atoms into First-Year Physics.

    ERIC Educational Resources Information Center

    Chabay, Ruth W.; Sherwood, Bruce A.

    1999-01-01

    Argues that thermal physics should not be treated as a separate topic in introductory physics. Provides an example of a course that emphasizes physical modeling of the phenomenon in terms of the atomic nature of matter. (Author/CCM)

  11. Atomic-orbital expansion model for describing ion-atom collisions at intermediate and low energies

    SciTech Connect

    Lin, C.D.; Fritsch, W.

    1983-01-01

    In the description of inelastic processes in ion-atom collisions at moderate energies, the semiclassical close-coupling method is well established as the standard method. Ever since the pioneering work on H/sup +/ + H in the early 60's, the standard procedure is to expand the electronic wavefunction in terms of molecular orbitals (MO) or atomic orbitals (AO) for describing collisions at, respectively, low or intermediate velocities. It has been recognized since early days that traveling orbitals are needed in the expansions in order to represent the asymptotic states in the collisions correctly. While the adoption of such traveling orbitals presents no conceptual difficulties for expansions using atomic orbitals, the situation for molecular orbitals is less clear. In recent years, various forms of traveling MO's have been proposed, but conflicting results for several well-studied systems have been reported.

  12. Reactive collisions of atomic antihydrogen with H, He+ and He

    NASA Astrophysics Data System (ADS)

    Cohen, James S.

    2006-03-01

    The fermion molecular dynamics (FMD) method is used to determine the rearrangement and destruction cross sections for collisions of antihydrogen (\\bar{H}) with H, He+ and He at collision energies above 0.1 au. The results for the H and He+ targets satisfactorily merge with previous calculations done for lower collision energies. Despite the absence of a critical distance, the destruction cross section for collisions of \\bar{H} with He, previously uncalculated, is found to be comparable with the destruction cross sections for \\bar{H} collisions with H and He+. All three cross sections are shown to be given quite reasonably by simple classical orbiting formulae at energies that are very low but still high enough for L > 0 partial waves to be dominant. The cross sections for formation of the antiprotonic atoms (Pn or \\barpHe ) and their initial quantum numbers with the \\bar{H} projectile are found to be significantly different from the analogous cross sections for \\barp projectiles.

  13. Atomic physics with highly charged ions

    SciTech Connect

    Richard, P.

    1991-08-01

    This report discusses: One electron outer shell processes in fast ion-atom collisions; role of electron-electron interaction in two-electron processes; multi-electron processes at low energy; multi-electron processes at high energy; inner shell processes; molecular fragmentation studies; theory; and, JRM laboratory operations.

  14. Physics through the 1990s: Atomic, molecular and optical physics

    NASA Technical Reports Server (NTRS)

    1986-01-01

    The volume presents a program of research initiatives in atomic, molecular, and optical physics. The current state of atomic, molecular, and optical physics in the US is examined with respect to demographics, education patterns, applications, and the US economy. Recommendations are made for each field, with discussions of their histories and the relevance of the research to government agencies. The section on atomic physics includes atomic theory, structure, and dynamics; accelerator-based atomic physics; and large facilities. The section on molecular physics includes spectroscopy, scattering theory and experiment, and the dynamics of chemical reactions. The section on optical physics discusses lasers, laser spectroscopy, and quantum optics and coherence. A section elucidates interfaces between the three fields and astrophysics, condensed matter physics, surface science, plasma physics, atmospheric physics, and nuclear physics. Another section shows applications of the three fields in ultra-precise measurements, fusion, national security, materials, medicine, and other topics.

  15. The Strange World of Ultracold Atomic Collisions: A Cornucopia of Quantum Phenomena

    NASA Astrophysics Data System (ADS)

    Williams, Carl J.

    1996-11-01

    The phenomenal experimental success of laser cooling and atom trapping has has helped to reinvigorate the field of atomic physics and has spawned the field of ultracold atomic collisions. This talk presents an overview of ultracold atomic collisions with an emphasis on some of the remarkable quantum phenomena -- including the Wigner threshold law -- that are inherent in these collisions. Additionally, we discuss the importance of ultracold collisions in Bose-Einstein condensation (BEC) of weakly interacting atomic systems and their role in the development of an atom laser and atomic clocks. Ultracold atomic collisions can be loosely broken into two classes of problems, collisions of ground state atoms (including metastable atoms) and the collision of atoms in external electric fields. In this latter class is the field of photoassociation spectroscopy. Theoretical analysis of the photoassociation spectrum of the Na2 purely long-range 0^-g state has recently produced three remarkable results. The first two results include the currently most accurate determination of the Na(3P) lifetime and the observation of the predicted but previously unobserved effect of retardation in the interaction between two atoms(K. M. Jones, P. S. Julienne, P. D. Lett, W. D. Phillips, E. Tiesinga, and C. J. Williams, Europhys. Lett. 35), 85 (1996).. Finally, the scattering length for the collision of two Na(3S) atoms in their F=1, M_F=-1 hyperfine state was extracted from the intensities and widths of the 0^-g spectra(E. Tiesinga, C. J. Williams, P. S. Julienne, K. M. Jones, P. D. Lett, and W. D. Phillips, J. Res. Nat. Inst. Stand. Technol. 101) (1996, in press).. Similar types of results have also been obtained in Li_2, K_2, and Rb_2. Ground state scattering lengths are essential for both modeling the formation of a BEC and for understanding collisional loss processes in a BEC. Similar collisional processes are important in pressure shifts in atomic clocks. We use the value of the of the

  16. The role of prompt electrons in the post-collision effect in fast ion - atom collisions

    NASA Astrophysics Data System (ADS)

    Víkor, Gy; Ricz, S.; Kövér, Á.; Gulyás, L.; Pelicon, P.; Sulik, B.

    1997-10-01

    The influence of the post-collision Coulomb effect of direct-electrons on the Auger-line energy shift has been studied in fast proton - atom collisions. KLL and LMM Auger spectra of neon and krypton target have been measured and analysed with high precision. The semiclassical theory of the post-collision interaction (PCI) has been extended to include the effect of both the receeding projectile ion and the ejected prompt electron. Experimental and theoretical line-energy shifts exhibit a reasonable agreement in the entire angular range of the Auger emission. In a narrow cone around 0953-4075/30/19/020/img9, the line-energy shift is influenced mainly by the PCI with the projectile ion, while at backward angles, it is predominantly governed by the ejected electron - Auger - electron interaction.

  17. ATOMIC AND MOLECULAR PHYSICS: Interference Angle on Quantum Rotational Energy Transfer in Na + Na2 (A1 Σ+u, v = 8 ~ b3п0u, v = 14) Molecular Collision System

    NASA Astrophysics Data System (ADS)

    Wang, Wei-Li; Miao, Gang; Li, Jian; Ma, Feng-Cai

    2009-12-01

    In order to study the collisional quantum interference (CQI) on rotational energy transfer in atom-diatom system, we have studied the relation of the integral interference angle and differential interference angle in Na + Na2 (A1 σ+u, v = 8 ~ b3п0u, v = 14) collision system. In this paper, based on the first-Born approximation of time-dependent perturbation theory and taking into accounts the anisotropic effect of Lennard-Jones interaction potentials, we present a theoretical model of collisional quantum interference in intramolecular rotational energy transfer, and a relationship between differential and integral interference angles.

  18. Atomic collisions with 33-TeV lead ions

    SciTech Connect

    Vane, C.R.; Datz, S.; Krause, H.F.

    1996-10-01

    Recent availability of relativistic and ultrarelativistic beams of heavy ions has permitted the first controlled studies of atomic collisions at energies sufficient to measure effects of several new basic phenomena. These include measurements substantiating recently predicted finite nuclear size effects resulting in a reduction in the total electronic energy loss of heavy ions in matter, and measurements of Coulomb collisions in which electrons are excited from the Dirac negative energy continuum. Measurements of total energy loss, free electron-positron pair production, and electron capture from pair production have been recently performed using 33-TeV Pb{sup 82+} ions from the CERN SPS accelerator in Geneva. Results of these studies are presented, along with comparisons with relevant theory.

  19. A distorted wave impulse approach for atom--diatom collisions

    SciTech Connect

    Dothe, H. ); Sharma, R.D. , Hanscom Air Force Base, Massachusetts 01731-5000 )

    1993-03-15

    A formalism is derived to include the effects of the long-range attractive part of the interaction potential in the calculation of atom--diatom collision cross sections using the impulse approach (IA). These calculations have, until now, assumed the atom--diatom potential given by a sum of two atom--atom interactions, consequently yielding a poor representation of the long-range attractive part. In the distorted wave impulse approach (DWIA) the long-range attractive part, located at the center of mass of the diatom, is a spherically symmetric potential which distorts'' the incoming and outgoing waves. The DWIA formalism is used to calculate differential cross sections for the rotationally inelastic process Li[sup +]+N[sub 2]([ital v]=0, [ital j]=2)[r arrow]Li[sup +]+N[sub 2]([ital v][prime]=0, [ital j][prime]), as a function of the final rotational level [ital j][prime], at a relative kinetic energy of 4.23 eV and center of mass scattering angles of 49.2[degree] and 37.1[degree]. It is shown that differential cross sections calculated using the DWIA formalism are in much better agreement with experimentally measured ones than IA differential cross sections using atom--atom interactions expressed by either hard-core, or exponential repulsive, functions.

  20. Theoretical atomic physics code development I: CATS: Cowan Atomic Structure Code

    SciTech Connect

    Abdallah, J. Jr.; Clark, R.E.H.; Cowan, R.D.

    1988-12-01

    An adaptation of R.D. Cowan's Atomic Structure program, CATS, has been developed as part of the Theoretical Atomic Physics (TAPS) code development effort at Los Alamos. CATS has been designed to be easy to run and to produce data files that can interface with other programs easily. The CATS produced data files currently include wave functions, energy levels, oscillator strengths, plane-wave-Born electron-ion collision strengths, photoionization cross sections, and a variety of other quantities. This paper describes the use of CATS. 10 refs.

  1. Relativistic atomic physics at the SSC

    SciTech Connect

    1990-12-31

    This report discusses the following proposed work for relativistic atomic physics at the Superconducting Super Collider: Beam diagnostics; atomic physics research; staffing; education; budget information; statement concerning matching funds; description and justification of major items of equipment; statement of current and pending support; and assurance of compliance.

  2. The Effect of Intense Laser Radiation on Atomic Collisions

    NASA Astrophysics Data System (ADS)

    Young, Stephen Michael Radley

    1991-02-01

    Available from UMI in association with The British Library. Requires signed TDF. We have carried out theoretical and experimental studies into the effect of intense laser radiation on atomic collisions. The first experiment used neon. Excitation by electron impact in a gas discharge demanded a pressure of at least 0.075 Torr. Measurement of the intensity of 3^1S_0to 3^1P_1 fluorescence has been made for the case where high intensity ASE wings in the laser profile and background laser scatter are unimportant, with the laser tuned to resonance. The field intensity required to produce strong field fluorescence (exemplified by the Mollow triplet) was found to give rise to complications capable of screening the effects sought. Our theoretical model has suggested that at finite detunings, line-centre fluorescence will dominate Rayleigh scatter and omega_3 fluorescence. Our measurements provide information on the saturation of neon fluorescence but not of the variation of the intense field collision rate. Absorption of weak field 253.7 nm laser photons by ground state mercury atoms yielded a high 6 ^3P_1 population at a lower pressure of 0.02 Torr. The Mollow triplet has been observed in the self-broadened mercury system. Dressing of the upper transition (6^3P_1rightarrow 7^3S_1) by an intense laser close to 435.8 nm yielded the strong field signal. Polarisation studies were made possible by the 3-level mercury system (radiation trapping in a 2-level system would depolarise fluorescence) perturbed by argon. The studies yielded results that were explainable in terms of the selective population of Stark shifted dressed states by a detuned, weak probe field. Use has been made of the electric-dipole radiation selection rule m_{J}=0 rightarrow m_{J^' } = 0 unless J=J^' to devise a 'Stark shift collision switch'. The competition between collision and radiation induced transitions within the mercury atom has then been studied. The resonant, strong lambda 435.8 nm field was used

  3. Atomic collision processes for modelling cool star spectra

    NASA Astrophysics Data System (ADS)

    Barklem, Paul

    2015-05-01

    The abundances of chemical elements in cool stars are very important in many problems in modern astrophysics. They provide unique insight into the chemical and dynamical evolution of the Galaxy, stellar processes such as mixing and gravitational settling, the Sun and its place in the Galaxy, and planet formation, to name a just few examples. Modern telescopes and spectrographs measure stellar spectral lines with precision of order 1 per cent, and planned surveys will provide such spectra for millions of stars. However, systematic errors in the interpretation of observed spectral lines leads to abundances with uncertainties greater than 20 per cent. Greater precision in the interpreted abundances should reasonably be expected to lead to significant discoveries, and improvements in atomic data used in stellar atmosphere models play a key role in achieving such advances in precision. In particular, departures from the classical assumption of local thermodynamic equilibrium (LTE) represent a significant uncertainty in the modelling of stellar spectra and thus derived chemical abundances. Non-LTE modelling requires large amounts of radiative and collisional data for the atomic species of interest. I will focus on inelastic collision processes due to electron and hydrogen atom impacts, the important perturbers in cool stars, and the progress that has been made. I will discuss the impact on non-LTE modelling, and what the modelling tells us about the types of collision processes that are important and the accuracy required. More specifically, processes of fundamentally quantum mechanical nature such as spin-changing collisions and charge transfer have been found to be very important in the non-LTE modelling of spectral lines of lithium, oxygen, sodium and magnesium.

  4. Coherence and correlations in fast ion-atom collisions

    SciTech Connect

    Burgdoerfer, J.

    1987-01-01

    This paper focusses on the description, classification and interpretation of coherent excitation of atomic or ionic systems with Coulombic two-body final state interactions. A group-theoretical approach is used to classify and interpret coherent excitation. The most significant result is that the state of excitation represented by a density operator can be mapped one to one onto expectation values of a set of operators. Examples are used to illustrate what can be learned about the collision process from investigations of coherent excitation. (JDH)

  5. The Screening Effect in Electromagnetic Production of Electron Positron Pairs in Relativistic Nucleus-Atom Collisions

    NASA Technical Reports Server (NTRS)

    Wu, Jianshi; Derrickson, J. H.; Parnell, T. A.; Strayer, M. R.

    1999-01-01

    We study the screening effects of the atomic electrons in the electromagnetic production of electron-positron pairs in relativistic nucleus-atom collisions for fixed target experiments. Our results are contrasted with those obtained in bare collisions, with particular attention given to its dependence on the beam energy and the target atom.

  6. Formation of positron-atom bound states in collisions between Rydberg Ps and neutral atoms

    NASA Astrophysics Data System (ADS)

    Swann, A. R.; Cassidy, D. B.; Deller, A.; Gribakin, G. F.

    2016-05-01

    Predicted 20 years ago, positron binding to neutral atoms has not yet been observed experimentally. A scheme is proposed to detect positron-atom bound states by colliding Rydberg positronium (Ps) with neutral atoms. Estimates of the charge-transfer reaction cross section are obtained using the first Born approximation for a selection of neutral atom targets and a wide range of incident Ps energies and principal quantum numbers. We also estimate the corresponding Ps ionization cross section. The accuracy of the calculations is tested by comparison with earlier predictions for charge transfer in Ps collisions with hydrogen and antihydrogen. We describe an existing Rydberg Ps beam suitable for producing positron-atom bound states and estimate signal rates based on the calculated cross sections and realistic experimental parameters. We conclude that the proposed methodology is capable of producing such states and of testing theoretical predictions of their binding energies.

  7. Multiple scattering and charged-particle - hydrogen-atom collisions

    NASA Technical Reports Server (NTRS)

    Franco, V.; Thomas, B. K.

    1979-01-01

    Glauber-approximation scattering amplitudes for charged-particle - hydrogen-atom elastic and inelastic collisions are derived directly in terms of the known particle-electron and particle-proton Coulomb scattering amplitudes and the known hydrogen-atom form factors. It is shown that the particle-hydrogen amplitude contains no single-scattering term. The double-scattering term is obtained as a two-dimensional integral in momentum space. It is demonstrated how the result can be used as the starting point for an alternative and relatively simple derivation, in closed form, of the Glauber particle-hydrogen scattering amplitude for transitions from the ground state to an arbitrary (nlm) state.

  8. Single electron capture in fast ion-atom collisions

    NASA Astrophysics Data System (ADS)

    Milojević, Nenad

    2014-12-01

    Single-electron capture cross sections in collisions between fast bare projectiles and heliumlike atomic systems are investigated by means of the four-body boundary-corrected first Born (CB1-4B) approximation. The prior and post transition amplitudes for single charge exchange encompassing symmetric and asymmetric collisions are derived in terms of twodimensional real integrals in the case of the prior form and five-dimensional quadratures for the post form. The dielectronic interaction V12 = 1/r12 = 1/|r1 - r2| explicitly appears in the complete perturbation potential Vf of the post transition probability amplitude T+if. An illustrative computation is performed involving state-selective and total single capture cross sections for the p - He (prior and post form) and He2+, Li3+Be4+B5+C6+ - He (prior form) collisions at intermediate and high impact energies. We have also studied differential cross sections in prior and post form for single electron transfer from helium by protons. The role of dynamic correlations is examined as a function of increased projectile energy. Detailed comparisons with the measurements are carried out and the obtained theoretical cross sections are in reasonable agreement with the available experimental data.

  9. Classical theory of atomic collisions - The first hundred years

    NASA Astrophysics Data System (ADS)

    Grujić, Petar V.

    2012-05-01

    Classical calculations of the atomic processes started in 1911 with famous Rutherford's evaluation of the differential cross section for α particles scattered on foil atoms [1]. The success of these calculations was soon overshadowed by the rise of Quantum Mechanics in 1925 and its triumphal success in describing processes at the atomic and subatomic levels. It was generally recognized that the classical approach should be inadequate and it was neglected until 1953, when the famous paper by Gregory Wannier appeared, in which the threshold law for the single ionization cross section behaviour by electron impact was derived. All later calculations and experimental studies confirmed the law derived by purely classical theory. The next step was taken by Ian Percival and collaborators in 60s, who developed a general classical three-body computer code, which was used by many researchers in evaluating various atomic processes like ionization, excitation, detachment, dissociation, etc. Another approach was pursued by Michal Gryzinski from Warsaw, who started a far reaching programme for treating atomic particles and processes as purely classical objects [2]. Though often criticized for overestimating the domain of the classical theory, results of his group were able to match many experimental data. Belgrade group was pursuing the classical approach using both analytical and numerical calculations, studying a number of atomic collisions, in particular near-threshold processes. Riga group, lead by Modris Gailitis [3], contributed considerably to the field, as it was done by Valentin Ostrovsky and coworkers from Sanct Petersbourg, who developed powerful analytical methods within purely classical mechanics [4]. We shall make an overview of these approaches and show some of the remarkable results, which were subsequently confirmed by semiclassical and quantum mechanical calculations, as well as by the experimental evidence. Finally we discuss the theoretical and

  10. Charge exchange and ionization in hydrogen atom-fully stripped ion collisions in Debye plasmas

    SciTech Connect

    Zhang, H.; Wang, J. G.; He, B.; Qiu, Y. B.; Janev, R. K.

    2007-05-15

    The processes of charge exchange and ionization in collisions of ground state hydrogen atom with fully stripped ions in a weakly coupled plasma are studied by the classical trajectory Monte Carlo method in the collision energy range 10-900 keV/amu. The interparticle interactions are described by the Debye-Hueckel model with inclusion of dynamical effects associated with the projectile velocity. The microcanonical distribution of initial state electronic coordinates and momenta has been determined by inclusion of plasma screening effects. The cross section dependencies on plasma parameters and ion charge and velocity are investigated. It is shown that plasma effects on charge exchange and ionization cross sections are significant and particularly pronounced at low collision velocities. The results of systematic cross section calculations for different values of Debye screening length (in the range 1-50a{sub 0}) and ion charges (in the range 1-14) are presented.

  11. Convergent Close-Coupling Approach to Electron-Atom Collisions

    NASA Technical Reports Server (NTRS)

    Bray, Igor; Stelbovics, Andris

    2007-01-01

    It was with great pleasure and honour to accept the invitation to make a presentation at the symposium celebrating the life-long work of Aaron Temkin and Richard Drachman. The work of Aaron Temkin was particularly influential on our own during the development of the CCC method for electron-atom collisions. There are a number of key problems that need to be dealt with when developing a general computational approach to such collisions. Traditionally, the electron energy range was subdivided into the low, intermediate, and high energies. At the low energies only a finite number of channels are open and variational or close-coupling techniques could be used to obtain accurate results. At high energies an infinite number of discrete channels and the target continuum are open, but perturbative techniques are able to yield accurate results. However, at the intermediate energies perturbative techniques fail and computational approaches need to be found for treating the infinite number of open channels. In addition, there are also problems associated with the identical nature of electrons and the difficulty of implementing the boundary conditions for ionization processes. The beauty of the Temkin-Poet model of electron-hydrogen scattering is that it simplifies the full computational problem by neglecting any non-zero orbital angular momenta in the partial-wave expansion, without loosing the complexity associated with the above-mentioned problems. The unique nature of the problem allowed for accurate solution leading to benchmark results which could then be used to test the much more general approaches to electron-atom collision problems. The immense value of the Temkin-Poet model is readily summarised by the fact that the initial papers of Temkin and Poet have been collectively cited around 250 times to date and are still being cited in present times. Many of the citations came from our own work during the course of the development of the CCC method, which we now describe.

  12. Collision lifetimes of polyatomic molecules at low temperatures: Benzene–benzene vs benzene–rare gas atom collisions

    SciTech Connect

    Cui, Jie; Krems, Roman V.; Li, Zhiying

    2014-10-28

    We use classical trajectory calculations to study the effects of the interaction strength and the geometry of rigid polyatomic molecules on the formation of long-lived collision complexes at low collision energies. We first compare the results of the calculations for collisions of benzene molecules with rare gas atoms He, Ne, Ar, Kr, and Xe. The comparison illustrates that the mean lifetimes of the collision complexes increase monotonically with the strength of the atom–molecule interaction. We then compare the results of the atom–benzene calculations with those for benzene–benzene collisions. The comparison illustrates that the mean lifetimes of the benzene–benzene collision complexes are significantly reduced due to non-ergodic effects prohibiting the molecules from sampling the entire configuration space. We find that the thermally averaged lifetimes of the benzene–benzene collisions are much shorter than those for Xe with benzene and similar to those for Ne with benzene.

  13. ANGULAR MOMENTUM CHANGING TRANSITIONS IN PROTON-RYDBERG HYDROGEN ATOM COLLISIONS

    SciTech Connect

    Vrinceanu, D.; Onofrio, R.; Sadeghpour, H. R. E-mail: onofrior@gmail.com

    2012-03-01

    Collisions between electrically charged particles and neutral atoms are central for understanding the dynamics of neutral gases and plasmas in a variety of physical situations of terrestrial and astronomical interest. Specifically, redistribution of angular momentum states within the degenerate shell of highly excited Rydberg atoms occurs efficiently in distant collisions with ions. This process is crucial in establishing the validity of the local thermal equilibrium assumption and may also play a role in determining a precise ionization fraction in primordial recombination. We provide an accurate expression for the non-perturbative rate coefficient of collisions between protons and H(nl) ending in a final state H(nl'), with n being the principal quantum number and l, l' the initial and final angular momentum quantum numbers, respectively. The validity of this result is confirmed by results of classical trajectory Monte Carlo simulations. Previous results, obtained by Pengelly and Seaton only for dipole-allowed transitions l {yields} l {+-} 1, overestimate the l-changing collisional rate coefficients approximately by a factor of six, and the physical origin of this overestimation is discussed.

  14. Correlated charge-changing ion-atom collisions. Progress report, March 16, 1991--March 15, 1992

    SciTech Connect

    Tanis, J.A.

    1992-04-01

    This report summarizes the progress and accomplishments in accelerator atomic physics research supported by DOE grant DE-FG02-87ER13778 from March 16, 1991 through March 15, 1992. This work involves the experimental investigation of fundamental atomic processes in collisions of charged projectiles with neutral targets or electrons, with particular emphasis on two-electron interactions and electron correlation effects. Processes involving combinations of excitation, ionization, and charge transfer are investigated utilizing coincidence techniques in which projectiles charge-changing events are associated with x-ray emission, target recoil ions, or electron emission. New results have been obtained for studies involving (1) resonant recombination of atomic ions, (2) double ionization of helium, and (3) continuum electron emission. Experiments were conducted using accelerators at the Lawrence Berkeley Laboratory, Argonne National Laboratory, Michigan State University, Western Michigan University, and the Institute of Nuclear Research, Debrecen, Hungary. Brief summaries of work completed and work in progress are given in this report.

  15. Making More-Complex Molecules Using Superthermal Atom/Molecule Collisions

    NASA Technical Reports Server (NTRS)

    Shortt, Brian; Chutjian, Ara; Orient, Otto

    2008-01-01

    A method of making more-complex molecules from simpler ones has emerged as a by-product of an experimental study in outer-space atom/surface collision physics. The subject of the study was the formation of CO2 molecules as a result of impingement of O atoms at controlled kinetic energies upon cold surfaces onto which CO molecules had been adsorbed. In this study, the O/CO system served as a laboratory model, not only for the formation of CO2 but also for the formation of other compounds through impingement of rapidly moving atoms upon molecules adsorbed on such cold interstellar surfaces as those of dust grains or comets. By contributing to the formation of increasingly complex molecules, including organic ones, this study and related other studies may eventually contribute to understanding of the origins of life.

  16. Toward a Physical Characterization of Raindrop Collision Outcome Regimes

    NASA Technical Reports Server (NTRS)

    Testik, F. Y.; Barros, Ana P.; Bilven, Francis L.

    2011-01-01

    A comprehensive raindrop collision outcome regime diagram that delineates the physical conditions associated with the outcome regimes (i.e., bounce, coalescence, and different breakup types) of binary raindrop collisions is proposed. The proposed diagram builds on a theoretical regime diagram defined in the phase space of collision Weber numbers We and the drop diameter ratio p by including critical angle of impact considerations. In this study, the theoretical regime diagram is first evaluated against a comprehensive dataset for drop collision experiments representative of raindrop collisions in nature. Subsequently, the theoretical regime diagram is modified to explicitly describe the dominant regimes of raindrop interactions in (We, p) by delineating the physical conditions necessary for the occurrence of distinct types of collision-induced breakup (neck/filament, sheet, disk, and crown breakups) based on critical angle of impact consideration. Crown breakup is a subtype of disk breakup for lower collision kinetic energy that presents distinctive morphology. Finally, the experimental results are analyzed in the context of the comprehensive collision regime diagram, and conditional probabilities that can be used in the parameterization of breakup kernels in stochastic models of raindrop dynamics are provided.

  17. Physical Limits on Atomic Resolution

    NASA Astrophysics Data System (ADS)

    van Dyck, D.; van Aert, S.; den Dekker, A. J.

    2004-02-01

    It is shown that the ultimate resolution is not limited by the bandwidth of the microscope but by the bandwidth (i.e., the scattering power) of the object. In the case of a crystal oriented along a zone axis, the scattering is enhanced by the channeling of the electrons. However, if the object is aperiodic along the beam direction, the bandwidth is much more reduced. A particular challenge are the amorphous objects. For amorphous materials, the natural bandwidth is that of the single atom and of the order of 1 [Angstrom capital A, ring][minus sign]1, which can be reached with the present generation of medium voltage microscopes without aberration correctors. A clear distinction is made between resolving a structure and refining, that is, between resolution and precision. In the case of an amorphous structure, the natural bandwidth also puts a limit on the number of atom coordinates that can be refined quantitatively. As a consequence, amorphous structures cannot be determined from one projection, but only by using atomic resolution tomography. Finally a theory of experiment design is presented that can be used to predict the optimal experimental setting or the best instrumental improvement. Using this approach it is suggested that the study of amorphous objects should be done at low accelerating voltage with correction of both spherical and chromatic aberration.

  18. Quasiclassical Methods for Ion Collisions with Two-Electron Atoms

    NASA Astrophysics Data System (ADS)

    Cohen, James S.

    1996-05-01

    Results of two generalizations of the classical-trajectory Monte Carlo (CTMC) method will be reported. The first is the model, termed CTMC-KW, originally proposed by Kirschbaum and Wilets(C. L. Kirschbaum and L. Wilets, Phys. Rev. A 21), 834 (1980). that achieves quasiclassical stability of multi-electron atoms via effective potentials motivated by the Heisenberg and Pauli principles. It was recently shown that this model gives fairly accurate binding energies for all atoms.(J. S. Cohen, Phys. Rev. A 51), 266 (1995) The second is a new model, termed CTMC-eb, that achieves stability via constraining potentials imposing lower bounds on the one-electron energies. The latter model is closer in spirit to the original CTMC method. Applications are made to single and double electron transfer and ionization cross sections for collisions of H^+, He^2+, and Li^3+ ions with the helium atom. All possible rearrangement processes are treated simultaneously and consistently. The cross sections will be compared with accurate experimental values.

  19. Charge Transfer and Dissociation in Collisions of Metal Clusters with Atoms

    NASA Astrophysics Data System (ADS)

    Bréchignac, C.; Cahuzac, Ph.; Concina, B.; Leygnier, J.; Ruiz, L. F.; Zarour, B.; Hervieux, P. A.; Hanssen, J.; Politis, M. F.; Martín, F.

    2002-10-01

    We present a combined theoretical and experimental study of charge transfer and dissociation in collisions of slow Li2+31 clusters with Cs atoms. We provide a direct quantitative comparison between theory and experiment and show that good agreement is found only when the exact experimental time of flight and initial cluster temperature are taken into account in the theoretical modeling. We demonstrate the validity of the simple physical image that consists in explaining evaporation as resulting from a collisional energy deposit due to cluster electronic excitation during charge transfer.

  20. Thermal relaxation of molecular oxygen in collisions with nitrogen atoms.

    PubMed

    Andrienko, Daniil A; Boyd, Iain D

    2016-07-01

    Investigation of O2-N collisions is performed by means of the quasi-classical trajectory method on the two lowest ab initio potential energy surfaces at temperatures relevant to hypersonic flows. A complete set of bound-bound and bound-free transition rates is obtained for each precollisional rovibrational state. Special attention is paid to the vibrational and rotational relaxations of oxygen as a result of chemically non-reactive interaction with nitrogen atoms. The vibrational relaxation of oxygen partially occurs via the formation of an intermediate NO2 complex. The efficient energy randomization results in rapid vibrational relaxation at low temperatures, compared to other molecular systems with a purely repulsive potential. The vibrational relaxation time, computed by means of master equation studies, is nearly an order of magnitude lower than the relaxation time in N2-O collisions. The rotational nonequilibrium starts to play a significant effect at translational temperatures above 8000 K. The present work provides convenient relations for the vibrational and rotational relaxation times as well as for the quasi-steady dissociation rate coefficient and thus fills a gap in data due to a lack of experimental measurements for this system. PMID:27394110

  1. Thermal relaxation of molecular oxygen in collisions with nitrogen atoms

    NASA Astrophysics Data System (ADS)

    Andrienko, Daniil A.; Boyd, Iain D.

    2016-07-01

    Investigation of O2-N collisions is performed by means of the quasi-classical trajectory method on the two lowest ab initio potential energy surfaces at temperatures relevant to hypersonic flows. A complete set of bound-bound and bound-free transition rates is obtained for each precollisional rovibrational state. Special attention is paid to the vibrational and rotational relaxations of oxygen as a result of chemically non-reactive interaction with nitrogen atoms. The vibrational relaxation of oxygen partially occurs via the formation of an intermediate NO2 complex. The efficient energy randomization results in rapid vibrational relaxation at low temperatures, compared to other molecular systems with a purely repulsive potential. The vibrational relaxation time, computed by means of master equation studies, is nearly an order of magnitude lower than the relaxation time in N2-O collisions. The rotational nonequilibrium starts to play a significant effect at translational temperatures above 8000 K. The present work provides convenient relations for the vibrational and rotational relaxation times as well as for the quasi-steady dissociation rate coefficient and thus fills a gap in data due to a lack of experimental measurements for this system.

  2. Treatment of Ion-Atom Collisions Using a Partial-Wave Expansion of the Projectile Wavefunction

    ERIC Educational Resources Information Center

    Wong, T. G.; Foster, M.; Colgan, J.; Madison, D. H.

    2009-01-01

    We present calculations of ion-atom collisions using a partial-wave expansion of the projectile wavefunction. Most calculations of ion-atom collisions have typically used classical or plane-wave approximations for the projectile wavefunction, since partial-wave expansions are expected to require prohibitively large numbers of terms to converge…

  3. Magneto-optical trapping and ultracold collisions of potassium atoms

    NASA Astrophysics Data System (ADS)

    Williamson, R. S., III; Walker, T.

    1995-08-01

    We present measurements of loading and loss rates for a vapor-cell optical trap of the two naturally occurring potassium isotopes 39 K and 41K. The unresolved excited-state hyperfine structure makes trapping of K fundamentally different from trapping of the other alkalis and leads to an enhanced loading rate. We measure the loading rate as a function of laser intensity, beam size, and detuning and find that the results are in reasonable agreement with a simple rate-equation model for the loading process. The dependence of the loss rate on trapped-atom density determines the contribution to the loss rates from excited-state collisions. We find a substantial difference between the collisional loss rates for the two isotopes.

  4. Cold Collision Frequency Shift in Two-Dimensional Atomic Hydrogen

    SciTech Connect

    Ahokas, J.; Jaervinen, J.; Vasiliev, S.

    2007-01-26

    We report a measurement of the cold collision frequency shift in atomic hydrogen gas adsorbed on the surface of superfluid {sup 4}He at T(less-or-similar sign)90 mK. Using two-photon electron and nuclear magnetic resonance in 4.6 T field we separate the resonance line shifts due to the dipolar and exchange interactions, both proportional to surface density {sigma}. We find the clock shift {delta}{nu}{sub c}=-1.0(1)x10{sup -7} Hz cm{sup -2}x{sigma}, which is about 100 times smaller than the value predicted by the mean field theory and known scattering lengths in the three-dimensional case.

  5. Atoms-for-Peace: A Galactic Collision in Action

    NASA Astrophysics Data System (ADS)

    2010-11-01

    European Southern Observatory astronomers have produced a spectacular new image of the famous Atoms-for-Peace galaxy (NGC 7252). This galactic pile-up, formed by the collision of two galaxies, provides an excellent opportunity for astronomers to study how mergers affect the evolution of the Universe. Atoms-for-Peace is the curious name given to a pair of interacting and merging galaxies that lie around 220 million light-years away in the constellation of Aquarius. It is also known as NGC 7252 and Arp 226 and is just bright enough to be seen by amateur astronomers as a very faint small fuzzy blob. This very deep image was produced by ESO's Wide Field Imager on the MPG/ESO 2.2-metre telescope at ESO's La Silla Observatory in Chile. A galaxy collision is one of the most important processes influencing how our Universe evolves, and studying them reveals important clues about galactic ancestry. Luckily, such collisions are long drawn-out events that last hundreds of millions of years, giving astronomers plenty of time to observe them. This picture of Atoms-for-Peace represents a snapshot of its collision, with the chaos in full flow, set against a rich backdrop of distant galaxies. The results of the intricate interplay of gravitational interactions can be seen in the shapes of the tails made from streams of stars, gas and dust. The image also shows the incredible shells that formed as gas and stars were ripped out of the colliding galaxies and wrapped around their joint core. While much material was ejected into space, other regions were compressed, sparking bursts of star formation. The result was the formation of hundreds of very young star clusters, around 50 to 500 million years old, which are speculated to be the progenitors of globular clusters. Atoms-for-Peace may be a harbinger of our own galaxy's fate. Astronomers predict that in three or four billion years the Milky Way and the Andromeda Galaxy will collide, much as has happened with Atoms-for-Peace. But don

  6. Atomic jet with ionization detection for laser spectroscopy of Rydberg atoms under collisions and fields

    NASA Astrophysics Data System (ADS)

    Philip, G.

    2008-03-01

    An efficient atomic jet setup offering many unprecedented advantages over a conventional heat pipe setup used in multi-photon spectroscopy, mainly of alkaline-earth metals, has been constructed by a scheme in which the sample material is encapsulated in a disposable cartridge oven located inside a thermally stabilised heat-pipe and is made to effuse in to a row of atomic beams merging to form a jet target. This novel scheme combines the advantages of both high density atomic beam with convenient geometry for orthogonal excitation and high sensitive ionisation detection capabilities of thermionic diodes, besides eliminating several problems inherent in the usual heat-pipe operation. Out of various designs, typical results are presented for a linear heat-pipe with vertical atomic jet used in two-photon spectroscopy of highly excited states of Sr I. Controlled excitations of both Rydberg and non-Rydberg states, which cannot otherwise be accessed from the ground state due to parity and spectroscopic selection rules, have been achieved by employing a weak electric field complimented by collisions. The atomic jet setup is also found very useful for the study of collisional broadening and shift of excited states and time evolution of Rydberg atoms.

  7. Theoretical studies relating to the interaction of radiation with matter: Atomic collision processes occurring in the presence of radiation fields

    NASA Astrophysics Data System (ADS)

    Berman, P. R.

    1981-09-01

    Work is reported in the areas of: Two-Level Atom and Radiation Pulse; Effects of Collisions on Atomic Coherences; Effects of Collisions on Zeeman Coherences; Collision Effects in Degenerate-Four-Wave-Mixing; and Dressed-Atom Picture in Laser Spectroscopy.

  8. Magnetic Slowing Down of Spin Relaxation due to Binary Collisions of Alkali-Metal Atoms with Buffer-Gas Atoms

    NASA Astrophysics Data System (ADS)

    Walter, D. K.; Griffith, W. M.; Happer, W.

    2002-03-01

    We report the first studies of magnetic decoupling of the spin relaxation of alkali-metal atoms due to binary collisions with buffer gases. When binary collisions are the dominant relaxation mechanism, the relaxation and its magnetic decoupling are well described by the S-damping rate ΓSD due to the spin-rotation interaction γN˙S, the spin exchange rate ΓEX for collisions between alkali atoms, and a new ``Carver rate'' ΓC, due to the pressure-shift interaction δAİS, which can substantially broaden the magnetic decoupling curve while having no influence on the zero-field rates.

  9. PREFACE: XXVII International Conference on Photonic, Electronic and Atomic Collisions (ICPEAC 2011)

    NASA Astrophysics Data System (ADS)

    Williams, I. D.; van der Hart, H. W.; McCann, J. F.; Crothers, D. S. F.

    2012-11-01

    The XXVII International Conference on Photonic, Electronic and Atomic Collisions was held at Queen's University Belfast, Northern Ireland, 27 July - 2 August 2011. Members of the Local Organising Committee were drawn from the School of Mathematics and Physics of Queen's University Belfast, the School of Physical Sciences at Dublin City University, the School of Physics at University College Dublin and the Department of Experimental Physics at the National University of Ireland, Maynooth. The Conference was attended by 566 participants with contributions from 54 countries. The meeting attracted 786 contributed papers for presentation in the poster sessions. The conference included 20 Special Reports selected from the contributed papers, and these are included in part 1 of this volume. During the meeting a total of 65 Progress Reports were also presented, and the authors invited to submit written versions of their talks (see Part 1). Of the total number of contributed papers, 663 are included as refereed abstracts in parts 2 to 15 of this volume of Journal of Physics: Conference Series. Part 1 of this volume includes detailed write-ups of the majority of plenary lectures, progress reports and special reports, constituting a comprehensive tangible record of the meeting, and is additionally published in hard-copy as the Conference Proceedings. There were 5 plenary lectures given by Margaret Murnane on Ultrafast processes in atomic dynamics; Chris Greene on Few-body highly-correlated dynamics; Michael Allan on Electron-molecule collisions; Yasunori Yamazaki on Antiproton and positron collisions and Thomas Stöhlker on Relativistic ion collisions. Ian Spielman, winner of the IUPAP Young Scientist Prize for 2011, gave a special lecture entitled Modifying interatomic interactions using Raman coupling: a tale of slowly colliding Bose-Einstein condensates. In addition an evening public lecture by Mike Baillie on How precise tree-ring dating raises issues concerning the

  10. Atomic Structure Calculations from the Los Alamos Atomic Physics Codes

    DOE Data Explorer

    Cowan, R. D.

    The well known Hartree-Fock method of R.D. Cowan, developed at Los Alamos National Laboratory, is used for the atomic structure calculations. Electron impact excitation cross sections are calculated using either the distorted wave approximation (DWA) or the first order many body theory (FOMBT). Electron impact ionization cross sections can be calculated using the scaled hydrogenic method developed by Sampson and co-workers, the binary encounter method or the distorted wave method. Photoionization cross sections and, where appropriate, autoionizations are also calculated. Original manuals for the atomic structure code, the collisional excitation code, and the ionization code, are available from this website. Using the specialized interface, you will be able to define the ionization stage of an element and pick the initial and final configurations. You will be led through a series of web pages ending with a display of results in the form of cross sections, collision strengths or rates coefficients. Results are available in tabular and graphic form.

  11. Polarized noble-gas atoms: A tool for fundamental physics

    SciTech Connect

    Chupp, T.E.

    1993-05-01

    Polarized noble gas atom samples suitable for a variety of experiments can be produced by spin exchange with laser optically pumped alkali-metal vapors. Most stable and even radioactive isotopes of He, Ne, Kr, Xe and Rn have been polarized, and the field has been paced, in part by laser developments and study of the atomic collision processes. I will focus on two kinds of application: (1) precision measurement of free precession frequencies to probe fundamental concepts such as CP violation, Local Lorentz Invariance and Linearity in Quantum Mechanics; (2) a polarized {sup 3}He target for electron scattering to extract information on the structure of the neutron. The precision measurement techniques take advantage of long coherence times (measured in hours for {sup 3}He and {sup 21}Ne) and large signal to noise ratios to measure frequency shifts with precision 10{sup -7} Hz in one hour. The polarized {sup 3}He target is used to measure asymmetries in deep inelastic electron scattering which are dominated by the neutron since the proton spins are approximately paired in the ground state of the nucleus. The spin dependent structure function of the neutron is an essential probe of the quark-parton structure of the nucleon. All of these investigations combine fundamental and particle physics motivation with atomic physics and precision measurement techniques in a way that spans many subfields of physics.

  12. Theory of phonon inelastic atom--surface scattering. I. Quantum mechanical treatment of collision dynamics

    SciTech Connect

    Choi, B.H.; Poe, R.T.

    1985-08-01

    We present a systematic formulation of the atom--surface scattering dynamics which includes the vibrational states of the atoms in the solid (phonons). The properties of the total scattering wave function of the system, a representation of the interaction potential matrix, and the characteristics of the independent physical solutions are all derived from the translational invariance of the full Hamiltonian. The scattering equations in the integral forms as well as the related Green functions were also obtained. The configurational representations of the Green functions, in particular, are quite different from those of the conventional scattering theory where the collision partners are spatially localized. Various versions of the integral expression of scattering, transition, and reactance matrices were also obtained. They are useful for introducing approximation schemes. From the present formulation, some specific theoretical schemes which are more realistic compared to those that have been employed so far and at the same time capable of yielding effective ab initio computation are derived in the following paper. The time reversal invariance and the microscopic reversibility of the atom--surface scattering were discussed. The relations between the in and outgoing scattering wave functions which are satisfied in the atom--surface system and important in the transition matrix methods were presented. The phonon annihilation and creation, and the adsorption and desorption of the atom are related through the time reversal invariance, and thus the microscopic reversibility can be tested by the experiment.

  13. Potential Energy Curves and Collisions Integrals of Air Components. 2; Interactions Involving Ionized Atoms

    NASA Technical Reports Server (NTRS)

    Stallcop, James R.; Partridge, Harry; Levin, Eugene; Langhoff, Stephen R. (Technical Monitor)

    1995-01-01

    Collision integrals are fundamental quantities required to determine the transport properties of the environment surrounding aerospace vehicles in the upper atmosphere. These collision integrals can be determined as a function of temperature from the potential energy curves describing the atomic and molecular collisions. Ab initio calculations provide a practical method of computing the required interaction potentials. In this work we will discuss recent advances in scattering calculations with an emphasis on the accuracy that is obtainable. Results for interactions of the atoms and ionized atoms of nitrogen and oxygen will be reviewed and their application to the determination of transport properties, such as diffusion and viscosity coefficients, will be examined.

  14. Guide to Laboratory Practicum in Atomic Physics

    NASA Astrophysics Data System (ADS)

    Burbulea, N. F.; Golban, G. N.; Scurtul, V. V.; Oleynik, V. A.

    1980-12-01

    The broshure represents a collection of 11 Laboratory works in Quantum Optics, Semiconductor, Atomic and Nuclear Physics for students of 2-nd years from Technical High Schools. A minimum of theoretical knowledges is given as well as a description of experimental installation (setup),a number of control questions and a task to be carried out is presented for every of the Laboratory work.

  15. Atomic and molecular physics at LURE

    SciTech Connect

    Morin, P.

    1994-08-01

    A short overview of the present research activity at LURE is given, in the field of atomic and molecular physics. Three selected examples are discussed in more detail and the {open_quotes}SOLEIL{close_quotes} project of a new French synchrotron facility is presented.

  16. Atomic data for astrophysics: improved collision strengths for Fe viii

    NASA Astrophysics Data System (ADS)

    Del Zanna, G.; Badnell, N. R.

    2014-10-01

    We describe, and present the results of, a new large-scale R-matrix scattering calculation for the electron collisional excitation of Fe viii. We first discuss the limitations of the previous calculations, in particular concerning some strong EUV lines observed in the solar corona by the Hinode EUV Imaging Spectrometer. We then present a new target which represents an improvement over the previous ones for this particularly complex ion. We developed a new method, based on the use of term energy corrections within the intermediate coupling frame transformation method, to calculate the collision strengths. We compare predicted and observed line intensities using laboratory and solar spectra, finding excellent agreement for all the main soft X-ray and extreme ultraviolet (EUV) transitions, using the present atomic data. In particular, we show that Fe viii EUV lines observed by Hinode EIS can now be used to provide reliable electron temperatures for the solar corona. The full dataset (energies, transition probabilities and rates) is only available in electronic form at our APAP website (http://www.apap-network.org) as well as at the CDS via anonymous ftp to http://cdsarc.u-strasbg.fr (ftp://130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/570/A56

  17. United Atom Rotational Coupling in Proton + Helium Collision

    NASA Astrophysics Data System (ADS)

    Wang, Chiiling

    United-atom 2p(sigma)-2p(pi) rotational coupling in asymmetric collisions is influenced by an avoided crossing between the 2p(sigma) and 2s(sigma) orbitals. This influence is studied using the HeH('+) system as a prototype. In (SIGMA)(,2)-(SIGMA)(,3)-(pi)(,1) three-state calculations, the time-dependent Schrodinger equation is solved numerically. Substantial population of the 2s(sigma) state is found, which disagrees with the estimates based on the Landau-Zener model. The (SIGMA)(,3) level is populated directly by transitions near the avoided crossing at b = 0.4 au and indirectly by (SIGMA)(,2)-(pi)(,1)-(SIGMA)(,3) rotational coupling for b > 0.4 au. The ratios of P(,(SIGMA)(,3))(b)/ P(,(SIGMA)(,3))(b) + P(,(pi)(,1))(b) are calculated and compared with Dr. R. Hippler's experimental data. A six-state calculation, in the basis of (SIGMA)(,1), (SIGMA)(,2), (SIGMA)(,3), (SIGMA)(,4), (pi)(,1) and (pi)(,2) molecular states, is also made. Cross sections and alignment and orientation parameters have been computed from the transition amplitudes for various energies.

  18. Non-thermal Dupree diffusivity and shielding effects on atomic collisions in astrophysical turbulent plasmas

    NASA Astrophysics Data System (ADS)

    Lee, Myoung-Jae; Jung, Young-Dae

    2016-02-01

    The influence of non-thermal Dupree turbulence and the plasma shielding on the electron-ion collision is investigated in astrophysical non-thermal Lorentzian turbulent plasmas. The second-order eikonal analysis and the effective interaction potential including the Lorentzian far-field term are employed to obtain the eikonal scattering phase shift and the eikonal collision cross section as functions of the diffusion coefficient, impact parameter, collision energy, Debye length and spectral index of the astrophysical Lorentzian plasma. It is shown that the non-thermal effect suppresses the eikonal scattering phase shift. However, it enhances the eikonal collision cross section in astrophysical non-thermal turbulent plasmas. The effect of non-thermal turbulence on the eikonal atomic collision cross section is weakened with increasing collision energy. The variation of the atomic cross section due to the non-thermal Dupree turbulence is also discussed.

  19. The physics of proton antiproton collisions

    SciTech Connect

    Shochet, M. )

    1991-12-03

    This paper contains information information on: accelerator and detector; QCD studies; studies of the electroweak force; The search for the top quark; {beta} physics at hadron colliders; and the search for exotic objects and prospects for the future.

  20. The ALADDIN atomic physics database system

    SciTech Connect

    Hulse, R.A. )

    1990-05-01

    ALADDIN is an atomic physics database system which has been developed in order to provide a broadly-based standard medium for the exchange and management of atomic data. ALADDIN consists of a data format definition together with supporting software for both interactive searches as well as for access to the data by plasma modeling and other codes. 8AB The ALADDIN system is designed to offer maximum flexibility in the choice of data representations and labeling schemes, so as to support a wide range of atomic physics data types and allow natural evolution and modification of the database as needs change. Associated dictionary files are included in the ALADDIN system for data documentation. The importance of supporting the widest possible user community was also central to be ALADDIN design, leading to the use of straightforward text files with concatentated data entries for the file structure, and the adoption of strict FORTRAN 77 code for the supporting software. This will allow ready access to the ALADDIN system on the widest range of scientific computers, and easy interfacing with FORTRAN modeling codes, user developed atomic physics codes and database, etc. This supporting software consists of the ALADDIN interactive searching and data display code, together with the ALPACK subroutine package which provides ALADDIN datafile searching and data retrieval capabilities to user's codes.

  1. Correlated charge-changing ion-atom collisions. Progress report, February 16, 1990--February 15, 1993

    SciTech Connect

    Tanis, J.A.

    1993-02-01

    This report summarizes the progress and accomplishments in accelerator atomic physics research supported by DOE grant DE-FG02-87ER13778 from February 16, 1990 through February 15, 1993. This work involves the experimental investigation of atomic interactions in collisions of charged projectiles with neutral targets or electrons, with particular emphasis on two-electron interactions and electron-correlation effects. The processes studied are of interest both from fundamental and applied points of view. In the latter case, results are obtained which are relevant to the understanding of laboratory and astrophysical plasmas, highly-excited (Rydberg) and continuum states of atoms and ions, atomic structure effects, the interaction of ions with surfaces, and the development of heavy-ion storage-rings. The results obtained have provided the basis for several M.A. thesis projects at Western Michigan and several Ph.D. dissertation projects are currently underway. Summaries of work completed and work in progress are given below in Section II. This research has resulted in 26 papers (in print and in press), 12 invited presentations at national and international meetings, and 28 contributed presentations as detailed in Section III.

  2. Efimov physics in {sup 6}Li atoms

    SciTech Connect

    Braaten, Eric; Hammer, H.-W.; Kang, Daekyoung; Platter, Lucas

    2010-01-15

    A new narrow three-atom loss resonance associated with an Efimov trimer crossing the three-atom threshold has recently been discovered in a many-body system of ultracold {sup 6}Li atoms in the three lowest hyperfine spin states at a magnetic field near 895 G. O'Hara and coworkers have used measurements of the three-body recombination rate in this region to determine the complex three-body parameter associated with Efimov physics. Using this parameter as the input, we calculate the universal predictions for the spectrum of Efimov states and for the three-body recombination rate in the universal region above 600 G where all three scattering lengths are large. We predict an atom-dimer loss resonance at 672+-2 G associated with an Efimov trimer disappearing through an atom-dimer threshold. We also predict an interference minimum in the three-body recombination rate at 759+-1 G where the three-spin mixture may be sufficiently stable to allow experimental study of the many-body system.

  3. Atomic Physics 15: Proceedings of the Fifteenth International Conference on Atomic Physics.

    NASA Astrophysics Data System (ADS)

    van Linden van den Heuvell, H. B.; Walraven, J. T. M.; Reynolds, M. W.

    1997-07-01

    The Table of Contents for the full book PDF is as follows: * Preface * Generation of a "Schrödinger cat" of radiation and observation of its decoherence * Synthesis of entangled states and quantum computing * Entangled states of atomic ions for quantum metrology and computation * Entanglement and indistinguishability: Coherence experiments with photon pairs and triplets * Atom optics as a testing ground for quantum chaos * Coherent ultra-bright XUV lasers and harmonics * Hollow atoms * Interdisciplinary experiments with polarized noble gases * The creation and study of Bose-Einstein condensation in a cold alkali vapor * oscopic quantum phenomena in trapped Bose-condensed gases * Doppler-free spectroscopy of trapped atomic hydrogen * QED and the ground state of helium * Towards coherent atomic samples using laser cooling * Bose-Einstein condensation of a weakly-interacting gas * Zeeman and his contemporaries: Dutch physics around 1900 * Zeeman's great discovery * The Zeeman effect: A tool for atom manipulation * The Zeeman effect a century later: New insights into classical physics * QED effects in few-electron high-Z systems * Lamb shift experiments on high-Z one- and two-electron systems * Fundamental constants of nature * Response of atoms in photonic lattices * Hydrogen-like systems and quantum electrodynamics * New experiments with atomic lattices bound by light * Bloch oscillations of atoms in an optical potential * Quantum decoherence and inertial sensing with atom interferometers * Quantum effects in He clusters * Atoms in super-intense radiation fields * Wave packet dynamics of excited atomic electrons in intense laser fields * Nonlinear laser-electron scattering * Comparing the antiproton and proton and progress toward cold antihydrogen * Author Index

  4. PREFACE: XXVIII International Conference on Photonic, Electronic and Atomic Collisions (ICPEAC 2013)

    NASA Astrophysics Data System (ADS)

    Xiao, Guoqing; Cai, Xiaohong; Ding, Dajun; Ma, Xinwen; Zhao, Yongtao

    2014-04-01

    The 28th International Conference on Photonic, Electronic and Atomic Collisions (XXVIII ICPEAC) was held by the Institute of Modern Physics, Chinese Academy of Sciences (IMP) on 24-30 July, 2013 in Lanzhou, China. The 444 conference participants came from 37 countries and/or regions. Five plenary lectures, more than 80 progress reports and special reports had been arranged according to the decision of the ICPEAC International General Committee. Meanwhile, more than 650 abstracts were selected as poster presentations. Before the conference, three highly distinguished scientists, Professor Joachim Burgdöorfer, Professor Hossein Sadeghpour and Professor Yasunori Yamazaki, presented tutorial lectures with the support of the IMP Branch of Youth Innovation Promotion Association, CAS (IMP-YIPA). During the conference, Professor Jianwei Pan from University of Sciences and Technology in China presented an enlightening public lecture on quantum communication. Furthermore, 2013 IUPAP Young Scientist Prize was awarded to Dr T Jahnke from Johann Wolfgang Goethe University of Germany. The Sheldon Datz Prize for an Outstanding Young Scientist Attending ICPEAC was awarded to Dr Diogo Almeida from University of Fribourg of Switzerland. As a biannual academic conference, ICPEAC is one of the most important international conferences on atomic and molecular physics. The topic of the conference covers the recent progresses in photonic, electronic, atomic, ionic, molecular, cluster collisions with matter. With a history back to 1958, ICPEAC came to China for the very first time. IMP has been preparing the conference six years before, ever since the ICPEAC International General Committee made the decision to hold the XXVIII ICPEAC in Lanzhou. This proceedings includes the papers of the two plenary lectures, 40 progress reports, 17 special reports and 337 posters, which were reviewed and revised according to the comments of the referees. The Local Organizing Committee would like to

  5. Handbook explaining the fundamentals of nuclear and atomic physics

    NASA Technical Reports Server (NTRS)

    Hanlen, D. F.; Morse, W. J.

    1969-01-01

    Indoctrination document presents nuclear, reactor, and atomic physics in an easy, straightforward manner. The entire subject of nuclear physics including atomic structure ionization, isotopes, radioactivity, and reactor dynamics is discussed.

  6. Unified treatment of hadronic annihilation and protonium formation in slow collisions of antiprotons with hydrogen atoms

    NASA Astrophysics Data System (ADS)

    Sakimoto, Kazuhiro

    2013-07-01

    Antiproton (p¯) collisions with hydrogen atoms, resulting in the hadronic process of particle-antiparticle annihilation and the atomic process of protonium (p¯p) formation (or p¯ capture), are investigated theoretically. As the collision energy decreases, the collision time required for the p¯ capture becomes necessarily longer. Then, there is the possibility that the p¯-p annihilation occurs significantly before the p¯ capture process completes. In such a case, one can no longer consider the annihilation decay separately from the p¯ capture process. The present study develops a rigorous unified quantum-mechanical treatment of the annihilation and p¯ capture processes. For this purpose, an R-matrix approach for atomic collisions is extended to have complex-valued R-matrix elements allowing for the hadronic annihilation. Detailed calculations are carried out at low collision energies ranging from 10-8 to 10-1 eV, and the annihilation and the p¯ capture (total and product-state selected) cross sections are reported. Consideration is given to the difference between the direct annihilation occurring during the collision and the annihilation of p¯p occurring after the p¯ capture. The present annihilation process is also compared with the annihilation in two-body p¯+p collisions.

  7. Theoretical studies relating to the interaction of radiation with matter: Atomic collision processes occurring in the presence of radiation fields

    NASA Astrophysics Data System (ADS)

    1980-10-01

    Work is reported in the areas of: (1) collisionally-aided radiative excitation; (2) model potential calculations in atom-field-radiation systems; (3) coherence effects in radiative collisions; (4) two level atom radiation pulse; (5) resonance fluorescence in three level systems; (6) modulation spectroscopy; and (7) effects of collisions on atomic coherences.

  8. V. S. Lebedev and I. L. Beigman, Physics of Highly Excited Atoms and Ions

    NASA Astrophysics Data System (ADS)

    Mewe, R.

    1999-07-01

    This book contains a comprehensive description of the basic principles of the theoretical spectroscopy and experimental spectroscopic diagnostics of Rydberg atoms and ions, i.e., atoms in highly excited states with a very large principal quantum number (n≫1). Rydberg atoms are characterized by a number of peculiar physical properties as compared to atoms in the ground or a low excited state. They have a very small ionization potential (∝1/n2), the highly excited electron has a small orbital velocity (∝1/n), the radius (∝n2) is very large, the excited electron has a long orbital period (∝n3), and the radiation lifetime is very long (∝n3-5). At the same time the R. atom is very sensitive to perturbations from external fields in collisions with charged and neutral targets. In recent years, R. atoms have been observed in laboratory and cosmic conditions for n up to ˜1000, which means that the size amounts to about 0.1 mm, ˜106 times that of an atom in the ground state. The scope of this monograph is to familiarize the reader with today's approaches and methods for describing isolated R. atoms and ions, radiative transitions between highly excited states, and photoionization and photorecombination processes. The authors present a number of efficient methods for describing the structure and properties of R. atoms and calculating processes of collisions with neutral and charged particles as well as spectral-line broadening and shift of Rydberg atomic series in gases, cool and hot plasmas in laboratories and in astrophysical sources. Particular attention is paid to a comparison of theoretical results with available experimental data. The book contains 9 chapters. Chapter 1 gives an introduction to the basic properties of R. atoms (ions), Chapter 2 is devoted to an account of general methods describing an isolated Rydberg atom. Chapter 3 is focussed on the recent achievements in calculations of form factors and dipole matrix elements of different types of

  9. High charge state, ion-atom collision experiments using accel-decel

    SciTech Connect

    Bernstein, E.M.; Clark, M.W.; Tanis, J.A.; Graham, W.G.

    1987-01-01

    Recent studies of /sub 16/S/sup 13 +/ + He collisions between 2.5 and 200 MeV, which were made using the accel-decel technique with the Brookhaven National Laboratory coupled MP tandem Van de Graaff accelerators, are discussed. Cross sections were measured for single electron-capture and -loss as well as K x rays correlated to electron-capture. Other planned ion-atom collision experiments requiring accel-decel are also presented. 18 refs., 3 figs.

  10. Dynamical resonant electron capture in atom surface collisions: H- formation in H-Al(111) collisions

    NASA Astrophysics Data System (ADS)

    Borisov, A. G.; Teillet-Billy, D.; Gauyacq, J. P.

    1992-05-01

    The formation of H- ion by grazing-angle collisions of hydrogen on an Al(111) surface is investigated with the newly developed coupled angular mode method. The capture process involves a dynamical resonant process induced by the collision velocity. All the resonance properties of the H- level in front of an Al(111) surface are determined: position, width, and angular distribution of ejected electrons. The results are shown to account for the recent observations on H- formation by Wyputta, Zimny, and Winter.

  11. Spin flip rates in collisions between muonic atoms

    SciTech Connect

    Bracci, L.; Chiccoli, C.; Pasini, P.; Fiorentini, G.; Melezhik, V.S.; Wozniak, J.

    1988-12-27

    We present the calculation of spin flip rates for a wide range of temperatures in the case of (d..mu..)-d, (p..mu..)-p and (t..mu..)-t collisions. The calculations have been performed in the framework of the adiabatic representation of the three-body problem.

  12. Low-energy collisions of O/sup 2+/ with atoms and molecules

    SciTech Connect

    Huq, M.S.; Champion, R.L.; Doverspike, L.D.

    1988-04-01

    Absolute total cross sections for single-electron capture have been measured for collisions of O/sup 2+/ ions with He, Ne, Ar, H/sub 2/, D/sub 2/, N/sub 2/, and O/sub 2/. The relative collision energies of these experiments range from approximately 3 to 400 eV. The electron-capture cross section for O/sup 2+/+He collisions is found to agree well with previous distorted-wave calculations. Capture cross sections are generally larger for molecular targets than for the atomic targets.

  13. Assessment of ion-atom collision data for magnetic fusion plasma edge modelling

    NASA Astrophysics Data System (ADS)

    Phaneuf, R. A.

    Cross-section data for ion-atom collision processes which play important roles in the edge plasma of magnetically-confined fusion devices are surveyed and reviewed. The species considered include H, He, Li, Be, C, O, Ne, Al, Si, Ar, Ti, Cr, Fe, Ni, Cu, Mo, W and their ions. The most important ion-atom collision processes occurring in the edge plasma are charge-exchange reactions. Excitation and ionization processes are also considered. The scope is limited to atomic species and to collision velocities corresponding to plasma ion temperatures in the 2 to 200 eV range. Sources of evaluated or recommended data are presented where possible, and deficiencies in the data base are indicated.

  14. Attosecond timing the ultrafast charge-transfer process in atomic collisions

    SciTech Connect

    Hu, S. X.

    2011-04-15

    By solving the three-dimensional, time-dependent Schroedinger equation, we have demonstrated that the ultrafast charge-transfer process in ion-atom collisions can be mapped out with attosecond extreme uv (xuv) pulses. During the dynamic-charge transfer from the target atom to the projectile ion, the electron coherently populates the two sites of both nuclei, which can be viewed as a 'short-lived' molecular state. A probing attosecond xuv pulse can instantly unleash the delocalized electron from such a ''transient molecule,'' so that the resulting photoelectron may exhibit a ''double-slit'' interference. On the contrary, either reduced or no photoelectron interference will occur if the attosecond xuv pulse strikes well before or after the collision. Therefore, by monitoring the photoelectron interference visibility, one can precisely time the ultrafast charge-transfer process in atomic collisions with time-delayed attosecond xuv pulses.

  15. The Los Alamos suite of relativistic atomic physics codes

    DOE PAGESBeta

    Fontes, C. J.; Zhang, H. L.; Jr, J. Abdallah; Clark, R. E. H.; Kilcrease, D. P.; Colgan, J.; Cunningham, R. T.; Hakel, P.; Magee, N. H.; Sherrill, M. E.

    2015-05-28

    The Los Alamos SuitE of Relativistic (LASER) atomic physics codes is a robust, mature platform that has been used to model highly charged ions in a variety of ways. The suite includes capabilities for calculating data related to fundamental atomic structure, as well as the processes of photoexcitation, electron-impact excitation and ionization, photoionization and autoionization within a consistent framework. These data can be of a basic nature, such as cross sections and collision strengths, which are useful in making predictions that can be compared with experiments to test fundamental theories of highly charged ions, such as quantum electrodynamics. The suitemore » can also be used to generate detailed models of energy levels and rate coefficients, and to apply them in the collisional-radiative modeling of plasmas over a wide range of conditions. Such modeling is useful, for example, in the interpretation of spectra generated by a variety of plasmas. In this work, we provide a brief overview of the capabilities within the Los Alamos relativistic suite along with some examples of its application to the modeling of highly charged ions.« less

  16. The Los Alamos suite of relativistic atomic physics codes

    SciTech Connect

    Fontes, C. J.; Zhang, H. L.; Jr, J. Abdallah; Clark, R. E. H.; Kilcrease, D. P.; Colgan, J.; Cunningham, R. T.; Hakel, P.; Magee, N. H.; Sherrill, M. E.

    2015-05-28

    The Los Alamos SuitE of Relativistic (LASER) atomic physics codes is a robust, mature platform that has been used to model highly charged ions in a variety of ways. The suite includes capabilities for calculating data related to fundamental atomic structure, as well as the processes of photoexcitation, electron-impact excitation and ionization, photoionization and autoionization within a consistent framework. These data can be of a basic nature, such as cross sections and collision strengths, which are useful in making predictions that can be compared with experiments to test fundamental theories of highly charged ions, such as quantum electrodynamics. The suite can also be used to generate detailed models of energy levels and rate coefficients, and to apply them in the collisional-radiative modeling of plasmas over a wide range of conditions. Such modeling is useful, for example, in the interpretation of spectra generated by a variety of plasmas. In this work, we provide a brief overview of the capabilities within the Los Alamos relativistic suite along with some examples of its application to the modeling of highly charged ions.

  17. Atomic physics at the Argonne PII ECR (electron cyclotron resonance) Ion Source

    SciTech Connect

    Dunford, R.W.; Berry, H.G.; Billquist, P.J.; Pardo, R.C.; Zabransky, B.J.; Bakke, E.; Groeneveld, K.O.; Hass, M.; Raphaelian, M.L.A.

    1987-01-01

    An atomic physics beam line has been set up at the Argonne PII ECR Ion Source. The source is on a 350-kV high-voltage platform which is a unique feature of particular interest in work on atomic collisions. We describe our planned experimental program which includes: measurement of state-selective electron-capture cross sections, studies of doubly-excited states, precision spectroscopy of few-electron ions, tests of quantum electrodynamics, and studies of polarization transfer using optically pumped polarized alkali targets. The first experiments will be measurements of cross sections for electron capture into specific nl subshells in ion-atom collisions. Our method is to observe the characteristic radiation emitted after capture using a VUV spectrometer. Initial data from these experiments are presented. 12 refs., 4 figs.

  18. Energy loss straggling in collisions of fast finite-size ions with atoms

    SciTech Connect

    Makarov, D. N. Matveev, V. I.

    2013-03-15

    The influence of ion size on straggling of energy losses by fast partially stripped ions is studied using the nonperturbative approach based on the eikonal approximation. It is shown that such a consideration of collisions of ions with complex atoms can lead to considerable corrections in calculating root-mean-square straggling of energy losses by fast ions compared to the results obtained for point ions. The root-mean-square straggling of energy losses are calculated for bromide and iodine ions in collisions with copper, silver, and aluminum atoms. It is shown that allowance for the size of the electron 'coat' of an ion noticeably improves the agreement with experimental data.

  19. Dissociative Excitation of Even States of Tin Atoms in e-SnCl2 Collisions

    NASA Astrophysics Data System (ADS)

    Smirnov, Yu. M.

    2001-12-01

    Dissociative excitation of even levels of tin atoms in collisions of slow electrons with tin dichloride molecules is studied experimentally. The levels studied belong to the configurations 5 s 25 pnp 1, 3 L ( n=6, 7; L= S, P, D) and 5 s 25 p 4 f. Absolute values of cross sections for dissociative excitation at the electron energy of 100 eV are 1.05-2.56 times greater than cross sections for excitation in electron-atom collisions at the energy of 50 eV.

  20. Theoretical study of resonances in low-energy collisions of three identical atoms

    NASA Astrophysics Data System (ADS)

    Yuen, Chi Hong; Kokoouline, Viatcheslav

    2016-05-01

    Resonances in low-energy collisions of three identical atoms are studied theoretically using hyperspherical coordinates. Two different methods are used and compared to determine positions and widths of three-body resonances: the complex absorbing potential and eigenchannel R-matrix approaches. Good agreement between the results of the two approaches is found. Cross sections for dimer formation in three-body recombination is determined. For this purpose the formula of Ref. is used (and re-derived). The developed code is applied to study collisions of three hydrogen atoms at low energies. Supported by the National Science Foundation, Grant No PHY-15-06391.

  1. Differential collision cross-sections for atomic oxygen

    NASA Technical Reports Server (NTRS)

    Torr, Douglas G.

    1991-01-01

    Differential collision cross-sections of O on N2 and other gases were measured to understand vehicle-environmental contamination effects in orbit. The following subject areas are also covered: groundbased scientific observations of rocket releases during NICARE-1; data compression study for the UVI; science priorities for UV imaging in the mid-1990's; and assessment of optimizations possible in UV imaging systems.

  2. Atomic physics at the advanced photon source

    SciTech Connect

    Berry, H.G.; Cowan, P.L.; Gemmell, D.S.

    1995-08-01

    Argonne`s 7-GeV synchrotron light source (APS) is expected to commence operations for research early in FY 1996. The Basic Energy Sciences Synchrotron Research Center (BESSRC) is likewise expected to start its research programs at that time. As members of the BESSRC CAT (Collaborative Access Team), we are preparing, together with atomic physicists from the University of Western Michigan, the University of Tennessee, and University of Notre Dame, to initiate a series of atomic physics experiments that exploit the unique capabilities of the APS, especially its high brilliance for photon energies extending from about 3 keV to more than 50 keV. Most of our early work will be conducted on an undulator beam line and we are thus concentrating on various aspects of that beam line and its associated experimental areas. Our group has undertaken responsibilities in such areas as hutch design, evaluation of undulator performance, user policy, interfacing and instrumentation, etc. Initial experiments will probably utilize existing apparatus. We are, however, planning to move rapidly to more sophisticated measurements involving, for example, ion-beam targets, simultaneous laser excitation, and the spectroscopy of emitted photons.

  3. Non-thermal Dupree diffusivity and shielding effects on atomic collisions in Lorentzian turbulent plasmas

    NASA Astrophysics Data System (ADS)

    Lee, Myoung-Jae; Jung, Young-Dae

    2016-05-01

    The influence of non-thermal Dupree turbulence and the plasma shielding on the electron-ion collision is investigated in Lorentzian turbulent plasmas. The second-order eikonal analysis and the effective interaction potential including the Lorentzian far-field term are employed to obtain the eikonal scattering phase shift and the eikonal collision cross section as functions of the diffusion coefficient, impact parameter, collision energy, Debye length and spectral index of the astrophysical Lorentzian plasma. It is shown that the non-thermal effect suppresses the eikonal scattering phase shift. However, it enhances the eikonal collision cross section in astrophysical non-thermal turbulent plasmas. The effect of non-thermal turbulence on the eikonal atomic collision cross section is weakened with increasing collision energy. The variation of the atomic cross section due to the non-thermal Dupree turbulence is also discussed. This research was supported by Nuclear Fusion Research Program through NRF funded by the Ministry of Science, ICT & Future Planning (Grant No. 2015M1A7A1A01002786).

  4. Accurate abundance analysis of late-type stars: advances in atomic physics

    NASA Astrophysics Data System (ADS)

    Barklem, Paul S.

    2016-05-01

    The measurement of stellar properties such as chemical compositions, masses and ages, through stellar spectra, is a fundamental problem in astrophysics. Progress in the understanding, calculation and measurement of atomic properties and processes relevant to the high-accuracy analysis of F-, G-, and K-type stellar spectra is reviewed, with particular emphasis on abundance analysis. This includes fundamental atomic data such as energy levels, wavelengths, and transition probabilities, as well as processes of photoionisation, collisional broadening and inelastic collisions. A recurring theme throughout the review is the interplay between theoretical atomic physics, laboratory measurements, and astrophysical modelling, all of which contribute to our understanding of atoms and atomic processes, as well as to modelling stellar spectra.

  5. Formation of heavy-Rydberg ion-pair states in Rydberg atom collisions with attaching targets

    NASA Astrophysics Data System (ADS)

    Wang, Changhao; Kelley, Michael; Buathong, Sitti; Dunning, F. Barry

    2014-05-01

    Electron transfer in collisions between K(np)Rydberg atoms and electron attaching molecules can lead to formation of heavy-Rydberg ion-pair states comprising a weakly-bound positive-negative ion pair orbiting at large internuclear separations. In the present work ion-pair states are created in a small collision cell and allowed to exit into an analysis region where their binding energy and velocity distributions are determined with the aid of electric-field-induced dissociation and a position sensitive detector. Ion pair production is analyzed using a Monte Carlo collision code that models both the initial Rydberg electron capture and the subsequent behavior of the product ion pair. The data demonstrate that collisions with SF6 and CCl4 lead to formation of long-lived ion pair states with a broad distribution of binding energies whose velocity distribution is strongly peaked in the forward direction. Research supported by the Robert A. Welch Foundation.

  6. Heavy-Rydberg ion-pair formation in collisions of Rydberg atoms with attaching targets

    NASA Astrophysics Data System (ADS)

    Wang, Changhao; Kelley, Michael; Dunning, F. Barry

    2012-06-01

    Collisions between K(np) Rydberg atoms and electron attaching targets can lead to the creation of heavy-Rydberg ion-pair states comprising a weakly-bound positive-negative ion pair orbiting at large internuclear separations. The lifetimes of such states and their correlation with binding energy and the channels available for decay, which can be controlled by varying n, the Rydberg atom velocity, and the target species, are being investigated. The ion-pair states are produced in a small collision cell and allowed to exit to form a beam that passes between a pair of electrodes where their number and binding energy distribution is determined by electric field induced dissociation. Ion-pair production is analyzed with the aid of a Monte Carlo collision code that models both initial Rydberg electron capture and the subsequent evolution of the product ion pair. Research supported by the Robert A Welch Foundation.

  7. Electronic spin-flipping collisions of hydrogen atoms

    SciTech Connect

    Zygelman, B.

    2010-03-15

    We present a unified multichannel approach to calculate electron spin-exchange and spin-flipping transition cross sections for collisions of H with H, H with T, and T with T. We use the theory to calculate the hyperfine quenching cross sections for collision energies that range from 1 mK to thermal temperatures. We show that spin-flipping transitions are induced by the splitting of the b {sup 3{Sigma}}{sub u} Born-Oppenheimer potential via the long-range magnetic interactions among electrons. We find that the spin-flipping cross sections in the tritium dimer are about a magnitude larger than that predicted by mass scaling the H-H cross sections. For the former, we show that the spin-exchange cross sections are several magnitudes larger, at cold temperatures, than that of the hydrogen system. We compare the results of the multichannel approach with those obtained using approximate methods such as the degenerate internal-state, the elastic, and Born approximations and discuss their respective range of validity.

  8. Measurement of doubly differential electron distributions induced by atomic collisions: Apparatus and related instrumental effects

    NASA Astrophysics Data System (ADS)

    Bernardi, G.; Suárez, S.; Fregenal, D.; Focke, P.; Meckbach, W.

    1996-05-01

    We describe the experimental setup at Centro Atómico Bariloche for the measurement of doubly differential electron distributions, in energy and angle of emission, induced by atomic collisions. We present detailed information about the performance of the equipment including a discussion of instrumental effects that could have affected the measured spectra.

  9. Orientational invariance of the rotational transition probability in the sudden approximation. [atom-molecule collisions

    NASA Technical Reports Server (NTRS)

    Stallcop, J. R.

    1974-01-01

    Semiclassical collisions of an atom with a rigid-rotor molecule are examined in the sudden approximation. The rotational transition probability is shown to be invariant with respect to the choice of orientation for the molecular coordinate system; this fact contradicts recently reported results of a computer analysis. The present analysis may lead to an improved interpretation of recent molecular beam measurements.

  10. Atomic physics and non-equilibrium plasmas

    SciTech Connect

    Weisheit, J.C.

    1986-04-25

    Three lectures comprise the report. The lecture, Atomic Structure, is primarily theoretical and covers four topics: (1) Non-relativistic one-electron atom, (2) Relativistic one-electron atom, (3) Non-relativistic many-electron atom, and (4) Relativistic many-electron atom. The lecture, Radiative and Collisional Transitions, considers the problem of transitions between atomic states caused by interactions with radiation or other particles. The lecture, Ionization Balance: Spectral Line Shapes, discusses collisional and radiative transitions when ionization and recombination processes are included. 24 figs., 11 tabs.

  11. Isotopic and Symmetry Effects in the Collision of Atomic Helium

    NASA Astrophysics Data System (ADS)

    Bouledroua, Moncef; Bouchelaghem, Fouzia; Tahar Bouazza, M.; Reggami, Lamia

    2006-11-01

    The thermophysical properties of a helium dilute gas at low and high temperatures are revisited with new and recent potential data points. The second virial coefficients are computed in order to assess the accuracy of the constructed He-He potentials. The results, mainly at high temperatures, are in a good agreement with the published values. The isotopic effects due to the presence of ^4He and ^3He atoms are also examined and the calculations of various transport parameters, namely diffusion, viscosity, and thermal conductivity, are extended to include the nuclear spins and the symmetry effects, which arise from the identity and indistinguishability of the colliding atoms.

  12. Developing new theoretical models of the formation of atomic collision cascades and subcascades in irradiated solids

    SciTech Connect

    Metelkin, E. V.; Ryazanov, A. I. Semenov, E. V.

    2008-09-15

    A new theoretical model is developed for the investigation of atomic collision cascades and subcascades in irradiated solids consisting of atoms of a single type. The model is based on an analytical description of the elastic collisions between moving atoms knocked out of the crystal lattice sites and the immobile atoms of the lattice. The description is based on the linear kinetic Boltzmann equation describing the retardation of primary recoil atoms (PRAs) in irradiated solids. The laws of conservation for the total number and the kinetic energy of moving atoms, which follow from the kinetic Boltzmann equation, are analyzed using the proposed model. An analytical solution is obtained for the stationary kinetic Boltzmann equation, which describes the retardation of PRAs for a given source responsible for their production. A kinetic equation for the moving atoms and the corresponding laws of conservation are also analyzed with allowance for the binding energy of atoms at the crystal lattice sites. A criterion for determining the threshold energy of subcascade formation in irradiated solids is formulated. Based on this criterion, the threshold energy of subcascade formation is calculated using the Thomas-Fermi potential. Formulas are presented for determining the mean size and number of subcascades formed in a solid as functions of the PRA energy.

  13. PREFACE: XXIX International Conference on Photonic, Electronic, and Atomic Collisions (ICPEAC2015)

    NASA Astrophysics Data System (ADS)

    Díaz, C.; Rabadán, I.; García, G.; Méndez, L.; Martín, F.

    2015-09-01

    The 29th International Conference on Photonic, Electronic and Atomic Collisions (XXIX ICPEAC) was held at the Palacio de Congresos ''El Greco'', Toledo, Spain, on 22-28 July, 2015, and was organized by the Universidad Autónoma de Madrid (UAM) and the Consejo Superior de Investigaciones Científicas (CSIC). ICPEAC is held biannually and is one of the most important international conferences on atomic and molecular physics. The topic of the conference covers the recent progresses in photonic, electronic, and atomic collisions with matter. With a history back to 1958, ICPEAC came to Spain in 2015 for the very first time. UAM and CSIC had been preparing the conference for six years, ever since the ICPEAC International General Committee made the decision to hold the XXIX ICPEAC in Toledo. The conference gathered 670 participants from 52 countries and attracted 854 contributed papers for presentation in poster sessions. Among the latter, 754 are presented in issues 2-12 of this volume of the Journal of Physics Conference Series. In addition, five plenary lectures, including the opening one by the Nobel laureate Prof. Ahmed H. Zewail and the lectures by Prof. Maciej Lewenstein, Prof. Paul Scheier, Prof. Philip H. Bucksbaum, and Prof. Stephen J. Buckman, 62 progress reports and 26 special reports were presented following the decision of the ICPEAC International General Committee. Detailed write-ups of most of the latter are presented in issue 1 of this volume, constituting a comprehensive tangible record of the meeting. On the occasion of the International Year of Light (IYL2015) and with the support of the Fundación Española para la Ciencia y la Tecnología (FECYT), the program was completed with two public lectures delivered by the Nobel laureate Prof. Serge Haroche and the Príncipe de Asturias laureate Prof. Pedro M. Echenique on, respectively, ''Fifty years of laser revolutions in physics'rquot; and ''The sublime usefulness of useless science''. Also a

  14. Reaction of associative ionization N +O →NO+ +e- at slow collisions of atoms

    NASA Astrophysics Data System (ADS)

    Golubkov, Maxim G.; Ozerov, Georgy K.; Adamson, Sergey O.; Golubkov, Gennady V.; Malyshev, Nikolay S.; Dementiev, Andrey I.

    2015-11-01

    The endothermic reaction of associative ionization of nitrogen and oxygen atoms was studied in the case of slow atom collisions in the framework of multichannel quantum defect theory. The diabatic potential energy curves of the NO molecule excited states were calculated using multireference configuration interaction methods implemented in MOLPRO package. It was shown that cross section dependence on the energy of the colliding atoms is in a good agreement with the experiment. The rate coefficient of the reaction was defined at the temperature 100K ⩽ T ⩽ 1000K range. The obtained data may be used for calculating the tiered kinetics of highly excited Rydberg state population in low-temperature plasma.

  15. Energy losses of fast heavy multiply charged structural ions in collisions with complex atoms

    NASA Astrophysics Data System (ADS)

    Matveev, V. I.; Sidorov, D. B.

    2007-07-01

    A nonperturbatve theory of energy losses of fast heavy multiply charged structural ions in collisions with neutral complex atoms is elaborated with allowance for simultaneous excitations of ionic and atomic electron shells. Formulas for the effective deceleration that are similar to the well-known Bethe-Bloch formulas are derived. By way of example, the energy lost by partially stripped U q+ ions (10 ≤ q ≤ 70) colliding with argon atoms and also the energy lost by Au, Pb, and Bi ions colliding with various targets are calculated. The results of calculation are compared with experimental data.

  16. An independent-atom-model description of ion-molecule collisions including geometric screening corrections

    NASA Astrophysics Data System (ADS)

    Lüdde, Hans Jürgen; Achenbach, Alexander; Kalkbrenner, Thilo; Jankowiak, Hans-Christian; Kirchner, Tom

    2016-04-01

    A new model to account for geometric screening corrections in an independent-atom-model description of ion-molecule collisions is introduced. The ion-molecule cross sections for net capture and net ionization are represented as weighted sums of atomic cross sections with weight factors that are determined from a geometric model of overlapping cross section areas. Results are presented for proton collisions with targets ranging from diatomic to complex polyatomic molecules. Significant improvement compared to simple additivity rule results and in general good agreement with experimental data are found. The flexibility of the approach opens up the possibility to study more detailed observables such as orientation-dependent and charge-state-correlated cross sections for a large class of complex targets ranging from biomolecules to atomic clusters.

  17. Laser Assisted Free-Free Transition in Electron - Atom Collision

    NASA Technical Reports Server (NTRS)

    Sinha, C.; Bhatia, A. K.

    2011-01-01

    Free-free transition is studied for electron-Hydrogen atom system in ground state at very low incident energies in presence of an external homogeneous, monochromatic and linearly polarized laser field. The incident electron is considered to be dressed by the laser in a non perturbative manner by choosing the Volkov solutions in both the channels. The space part of the scattering wave function for the electron is solved numerically by taking into account the effect of electron exchange, short range as well as of the long range interactions. Laser assisted differential as well as elastic total cross sections are calculated for single photon absorption/emission in the soft photon limit, the laser intensity being much less than the atomic field intensity. A strong suppression is noted in the laser assisted cross sections as compared to the field free situations. Significant difference is noted in the singlet and the triplet cross sections.

  18. Broad Feshbach resonances in collisions of Dy atoms

    NASA Astrophysics Data System (ADS)

    Julienne, P.; Jachymski, K.; Maier, T.; Ferrier-Barbut, I.; Karan, H.; Schmitt, M.; Wenzel, M.; Wink, C.; Pfau, T.

    2016-05-01

    RF spectroscopy of weakly bound dimers of ultra cold bosonic Dy atoms gives evidence for the emergence of a universal s-wave halo state in a background of chaotic background resonance states. The halo state is associated with a broad magnetic Feshbach resonance. Using a coupled channels theory taking into account the short ranged van dear Waals interaction and a correction due to the strong dipole moment of Dy, we are able to extract the scattering length as a function of magnetic field tuning near two such broad resonances. These results offer prospects for tuning the interactions of Dy atoms in a regime where three-body losses are not too strong. Supported in part by the DFG, the Foundation for Polish Science International Ph. D Projects Programme, and an AFOSR MURI.

  19. Reactive collisions of atomic antihydrogen with H, He^+, He, H2^+, and H2

    NASA Astrophysics Data System (ADS)

    Cohen, James S.

    2006-05-01

    The fermion molecular dynamics (FMD) method has been used to determine the rearrangement and destruction cross sections for collisions of antihydrogen (H) with H, He^+, He, H2^+, and H2 at collision energies above 0.1 au. The results for the H and He^+ targets satisfactorily merge with previous calculations done for lower collision energies. There are no previous calculations for the other targets. Despite the absence of a critical distance, the destruction cross section for collisions of H with He is found to be comparable with the destruction cross sections for H collisions with H and He^+, for which there are critical distances. The three atomic cross sections are shown to be given quite reasonably by simple classical orbiting formulas at energies that are very low but still high enough for L>0 partial waves to be dominant. The cross sections for formation of the antiprotonic atoms (Pn or pHe) and their initial quantum numbers are found to be significantly different from the analogous cross sections for p projectiles. The cross sections for the molecular targets are significantly larger.

  20. Electron transfer, ionization, and excitation in atomic collisions. Progress report, June 15, 1992--June 14, 1995

    SciTech Connect

    Winter, T.G.; Alston, S.G.

    1995-08-01

    The research program of Winter and Alston addresses the fundamental processes of electron transfer, ionization, and excitation in ion-atom, ion-ion, and ion-molecule collisions. Attention is focussed on one- and two-electron systems and, more recently, quasi-one-electron systems whose electron-target-core interaction can be accurately modeled by one-electron potentials. The basic computational approaches can then be taken with few, if any, approximations, and the underlying collisional mechanisms can be more clearly revealed. Winter has focussed on intermediate collision energies (e.g., proton energies for p-He{sup +} collisions on the order of 100 kilo-electron volts), in which many electron states are strongly coupled during the collision and a coupled-state approach, such as a coupled-Sturmian-pseudostate approach, is appropriate. Alston has concentrated on higher collision energies (million electron-volt energies), or asymmetric collision systems, for which the coupling of the projectile is weaker with, however, many more target states being coupled together so that high-order perturbation theory is essential. Several calculations by Winter and Alston are described, as set forth in the original proposal.

  1. Project Physics Text 5, Models of the Atom.

    ERIC Educational Resources Information Center

    Harvard Univ., Cambridge, MA. Harvard Project Physics.

    Basic atomic theories are presented in this fifth unit of the Project Physics text for use by senior high students. Chemical basis of atomic models in the early years of the 18th Century is discussed n connection with Dalton's theory, atomic properties, and periodic tables. The discovery of electrons is described by using cathode rays, Millikan's…

  2. Delta-ray production in ion-atom collisions

    SciTech Connect

    Wilson, W.E.; Toburen, L.H.

    1980-07-01

    The stochastic energy concentrations randomly deposited in submicron volumes in and near the paths of charged particles is needed. Computational methods, especially Monte Carlo methods, required a comprehensive set of basic interaction cross sections for the primary and all secondary radiation products. Of particular importance for high LET radiations are the cross sections for the production of energetic secondary electrons, delta-rays, in primary ionizing events. In this paper, we review the present state of available data on the production of delta-rays by fast positive ions in collision with targets of biological interest. The systematics in the cross sections for proton ionization of molecular targets are discussed, indicating what scaling is possible and summarizing what can be concluded regarding the dependence of the mean delta-ray energies on the chemical makeup of the medium. A comparison of typical data is made with the binary-encounter approximation to illustrate the limitations of this theoretical treatment of the ionization process. A bibliography of relevant published works on this topic is included.

  3. Electron collisions with atoms, ions, molecules, and surfaces: Fundamental science empowering advances in technology.

    PubMed

    Bartschat, Klaus; Kushner, Mark J

    2016-06-28

    Electron collisions with atoms, ions, molecules, and surfaces are critically important to the understanding and modeling of low-temperature plasmas (LTPs), and so in the development of technologies based on LTPs. Recent progress in obtaining experimental benchmark data and the development of highly sophisticated computational methods is highlighted. With the cesium-based diode-pumped alkali laser and remote plasma etching of Si3N4 as examples, we demonstrate how accurate and comprehensive datasets for electron collisions enable complex modeling of plasma-using technologies that empower our high-technology-based society. PMID:27317740

  4. GENERAL VIEW, LOOKING NORTH, OF ATOMIC PHYSICS OBSERVATORY WHICH CONTAINS ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    GENERAL VIEW, LOOKING NORTH, OF ATOMIC PHYSICS OBSERVATORY WHICH CONTAINS THE WHITE DOME STRUCTURE. THE SHED-LIKE STRUCTURE TO THE LEFT IS THE SEARCH-LIGHT BUILDING. - Carnegie Institution of Washington, Department of Terrestrial Magnetism, Atomic Physics Observatory, 5241 Broad Branch Drive Northwest, Washington, District of Columbia, DC

  5. Multiple-ionization channels in proton-atom collisions

    SciTech Connect

    DuBois, R.D.; Manson, S.T.

    1987-03-01

    A detailed investigation of multiple ionization of He (ionization charge states q = 1,2), Ne (q = 1--3), and Ar and Kr (q = 1--4) is presented for proton impact energies ranging from 10 keV to a few MeV. Absolute cross sections for various ionization pathways have been obtained by combining some new measurements with previously published experimental results and, in certain cases, with existing theoretical information. It is shown how each of these pathways contribute to the various stages of target ionization that are observed after the collision and how these experimentally measured quantities are related to the cross sections for initial inner- and outer-shell vacancy production. Areas where additional data are required or where the existing data are not internally consistent are pointed out. In general, it is shown that the existing data are sufficient to describe the ionization of helium as well as the lower levels of ionization of neon, argon, and krypton. However, for the higher degrees of ionization, particularly for Kr, our understanding is hampered by substantial gaps in the available inner-shell ionization data: both in cross-section and branching-ratio information. Nevertheless, the data are sufficient to indicate the relative importance of the various pathways. For all targets, direct multiple outer-shell cross sections were extracted. Analyzing the energy dependences of these cross sections provided some hints as to how to calculate multiple-ionization cross sections, e.g., information as to where the multiple ionization is dominated by the first-order or by a higher-order term in the perturbation expansion of the proton-target interaction is obtained.

  6. Atomic Physics, Science (Experimental): 5318.42.

    ERIC Educational Resources Information Center

    Petit, Ralph E.

    Presented is the study of modern and classical concepts of the atom; the structure of the atom as a mass-energy relationship; practical uses of radioactivity; isotopes; and the strange particles. Performance objectives (16) are included as well as a detailed course outline. Experiments, demonstrations, projects and reports to enhance student…

  7. Inelastic scattering in atom-diatomic molecule collisions. I - Rotational transitions in the sudden approximation

    NASA Technical Reports Server (NTRS)

    Stallcop, J. R.

    1974-01-01

    The impact parameter method and the sudden approximation are applied to determine the total probability of inelastic rotational transitions arising from a collision of an atom and a homonuclear diatomic molecule at large impact parameters. An analytical approximation to this probability is found for conditions where the electron exchange or overlap forces dominate the scattering. An approximate upper bound to the range of impact parameters for which rotational scattering can be important is determined. In addition, an estimate of the total inelastic cross section is found at conditions for which a statistical model describes the scattering well. The results of this analysis are applied to Ar-O2 collisions and may be readily applied to other combinations of atoms and molecules.

  8. Ion-biomolecule collisions studied within the independent atom model including geometric screening corrections

    NASA Astrophysics Data System (ADS)

    Lüdde, H. J.; Achenbach, A.; Kalkbrenner, T.; Jankowiak, H. C.; Kirchner, T.

    2016-05-01

    A recently introduced model to account for geometric screening corrections in an independent-atom-model description of ion-molecule collisions is applied to proton collisions from amino acids and DNA and RNA nucleobases. The correction coefficients are obtained from using a pixel counting method (PCM) for the exact calculation of the effective cross sectional area that emerges when the molecular cross section is pictured as a structure of (overlapping) atomic cross sections. This structure varies with the relative orientation of the molecule with respect to the projectile beam direction and, accordingly, orientation-independent total cross sections are obtained from averaging the pixel count over many orientations. We present net capture and net ionization cross sections over wide ranges of impact energy and analyze the strength of the screening effect by comparing the PCM results with Bragg additivity rule cross sections and with experimental data where available. Work supported by NSERC, Canada.

  9. Atomic physics: A milestone in quantum computing

    NASA Astrophysics Data System (ADS)

    Bartlett, Stephen D.

    2016-08-01

    Quantum computers require many quantum bits to perform complex calculations, but devices with more than a few bits are difficult to program. A device based on five atomic quantum bits shows a way forward. See Letter p.63

  10. Tight Binding Models in Cold Atoms Physics

    NASA Astrophysics Data System (ADS)

    Zakrzewski, J.

    2007-05-01

    Cold atomic gases placed in optical lattice potentials offer a unique tool to study simple tight binding models. Both the standard cases known from the condensed matter theory as well as novel situations may be addressed. Cold atoms setting allows for a precise control of parameters of the systems discussed, stimulating new questions and problems. The attempts to treat disorder in a controlled fashion are addressed in detail.

  11. A model for energy transfer in collisions of atoms with highly excited molecules.

    PubMed

    Houston, Paul L; Conte, Riccardo; Bowman, Joel M

    2015-05-21

    A model for energy transfer in the collision between an atom and a highly excited target molecule has been developed on the basis of classical mechanics and turning point analysis. The predictions of the model have been tested against the results of trajectory calculations for collisions of five different target molecules with argon or helium under a variety of temperatures, collision energies, and initial rotational levels. The model predicts selected moments of the joint probability distribution, P(Jf,ΔE) with an R(2) ≈ 0.90. The calculation is efficient, in most cases taking less than one CPU-hour. The model provides several insights into the energy transfer process. The joint probability distribution is strongly dependent on rotational energy transfer and conservation laws and less dependent on vibrational energy transfer. There are two mechanisms for rotational excitation, one due to motion normal to the intermolecular potential and one due to motion tangential to it and perpendicular to the line of centers. Energy transfer is found to depend strongly on the intermolecular potential and only weakly on the intramolecular potential. Highly efficient collisions are a natural consequence of the energy transfer and arise due to collisions at "sweet spots" in the space of impact parameter and molecular orientation. PMID:25907301

  12. Atomic collisions in the presence of laser radiation - Time dependence and the asymptotic wave function

    NASA Technical Reports Server (NTRS)

    Devries, P. L.; George, T. F.

    1982-01-01

    A time-dependent, wave-packet description of atomic collisions in the presence of laser radiation is extracted from the more conventional time-independent, stationary-state description. This approach resolves certain difficulties of interpretation in the time-independent approach which arise in the case of asymptotic near resonance. In the two-state model investigated, the approach predicts the existence of three spherically scattered waves in this asymptotically near-resonant case.

  13. Inelastic scattering in atom-diatomic molecule collisions. II - Effect of rotation on vibrational transition

    NASA Technical Reports Server (NTRS)

    Stallcop, J. R.

    1975-01-01

    Rotational and vibrational transitions in a diatomic molecule caused by collisions with an atom are analyzed by a semiclassical method for conditions where the rotational transitions can be handled well by the sudden approximation and the vibrational transitions belong to the adiabatic regime. The contribution to the vibrational transition probability from the correction, which takes the finite value of the spacing between rotational energy levels into account, is examined.-

  14. Rotational excitation of hydrogen molecules by collisions with hydrogen atoms. [interstellar gas energetics

    NASA Technical Reports Server (NTRS)

    Green, S.; Truhlar, D. G.

    1979-01-01

    Rate constants for rotational excitation of hydrogen molecules by collisions with hydrogen atoms have been obtained from quantum-mechanical calculations for kinetic temperatures between 100 and 5000 K. These calculations involve the rigid-rotator approximation, but other possible sources of error should be small. The calculations indicate that the early values of Nishimura are larger than accurate rigid-rotator values by about a factor of 20 or more.

  15. Quantum-mechanical theory including angular momenta analysis of atom-atom collisions in a laser field

    NASA Technical Reports Server (NTRS)

    Devries, P. L.; George, T. F.

    1978-01-01

    The problem of two atoms colliding in the presence of an intense radiation field, such as that of a laser, is investigated. The radiation field, which couples states of different electronic symmetry, is described by the number state representation while the electronic degrees of freedom (plus spin-orbit interaction) are discussed in terms of a diabatic representation. The total angular momentum of the field-free system and the angular momentum transferred by absorption (or emission) of a photon are explicitly considered in the derivation of the coupled scattering equations. A model calculation is discussed for the Xe + F collision system.

  16. Nonadiabatic coupling in cold collisions of spin-polarized metastable hydrogen atoms

    SciTech Connect

    Forrey, Robert C.; Dalgarno, Alex; Vanne, Yulian V.; Saenz, Alejandro; Froelich, Piotr

    2007-11-15

    Previous calculations of low-temperature cross sections for collisions between spin-polarized metastable hydrogen atoms are improved to include nonadiabatic radial and angular coupling at large interatomic separations. The electrostatic dipole-quadrupole interaction produces nonadiabatic radial coupling between (2s,2p) and (2p,2p) states, while the Coriolis interaction produces nonadiabatic angular coupling. Both of these long-range contributions are handled in a space-fixed atomic gauge that is particularly convenient for a spin-polarized system. The improved theoretical results are compared with an existing experiment.

  17. Electron excitation collision strengths for positive atomic ions: a collection of theoretical data

    SciTech Connect

    Merts, A.L.; Mann, J.B.; Robb, W.D.; Magee, N.H. Jr.

    1980-03-01

    This report contains data on theoretical and experimental cross sections for electron impact excitation of positive atomic ions. It is an updated and corrected version of a preliminary manuscript which was used during an Atomic Data Workshop on Electron Excitation of Ions held at Los Alamos in November 1978. The current status of quantitative knowledge of collisional excitation collision strengths is shown for highly stripped ions where configuration mixing, relativistic and resonance effects may be important. The results show a reasonably satisfactory state for first-row isoelectronic ions and indicate that a considerable amount of work remains to be done for second-row and heavier ions.

  18. On the relativistic and nonrelativistic electron descriptions in high-energy atomic collisions

    NASA Astrophysics Data System (ADS)

    Voitkiv, A. B.

    2007-07-01

    We consider the relativistic and nonrelativistic descriptions of an atomic electron in collisions with point-like charged projectiles moving at relativistic velocities. We discuss three different forms of the fully relativistic first-order transition amplitude. Using the Schrödinger-Pauli equation to describe the atomic electron we establish the correct form of the nonrelativistic first-order transition amplitude. We also show that the so-called semi-relativistic treatment, in which the Darwin states are used to describe the atomic electron, is in fact fully equivalent to the nonrelativistic consideration. The comparison of results obtained with the relativistic and nonrelativistic electron descriptions shows that the latter is accurate within 20-30% up to Za<~ 50-60, where Za is the atomic nuclear charge.

  19. Detecting high-density ultracold molecules using atom-molecule collision

    NASA Astrophysics Data System (ADS)

    Chen, Jun-Ren; Kao, Cheng-Yang; Chen, Hung-Bin; Liu, Yi-Wei

    2013-04-01

    Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecules utilizing inelastic atom-molecule collision is demonstrated. The resonant coupling effect on the formation of the X1Σ+g ground state 85Rb2 allows for a sufficient number of more deeply bound ultracold molecules, which induced an additional trap loss and heating of the co-existing atoms owing to the inelastic atom-molecule collision. Therefore, after the photoassociation process, the ultracold molecules can be investigated using the absorption image of the ultracold rubidium atoms mixed with the molecules in a crossed optical dipole trap. The existence of the ultracold molecules was then verified, and the amount of accumulated molecules was measured. This method detects the final produced ultracold molecules, and hence is distinct from the conventional trap loss experiment, which is used to study the association resonance. It is composed of measurements of the time evolution of an atomic cloud and a decay model, by which the number density of the ultracold 85Rb2 molecules in the optical trap was estimated to be >5.2 × 1011 cm-3.

  20. Charge transfer in slow collisions between hydrogen atoms and metal surfaces

    NASA Astrophysics Data System (ADS)

    Bahrim, B.; Thumm, U.

    2002-05-01

    We have developed a new two-center close-coupling approach [1] for slow ion (atom)-surface collision in which the continuum of metal conduction-band states is discretized by using Weyl wave packets [2] to represent the motion of the active electron in the metal subspace. Results for the time evolution of the atomic and metallic population amplitudes for a hydrogen atom in colliding at perpendicular incidence with an model aluminum surface are shown and discussed. For the n=2 hydrogenic manifold, we have obtained converged atomic populations amplitudes by including all projectile levels up to the n=5 manifold and 480 Weyl wave packets in the close-coupling expansion. We will discuss the electron dynamics in particular in view of possible dephasing effects (in distance and time) and recurrence effects that may arrise due to our continuum discretization in term of a finite number of localized Weyl packets. [1] B. Bahrim and U. Thumm, Surf. Sci. 451, 1 (2000), and to appear in Phys. Rev. A. [2] B.H. Bransden and M.R.C. McDowell, "Charge Exchange and the Theory of Ion-Atom Collisions" Clarendon Press (Oxford 1992). Supported by NSF and by the Division of Chemical Sciences, Office of Basic Energy Sciences, Office of Energy Research, U.S. DOE

  1. Investigation of cold collision in a two isotope magneto-optical trap for Krypton atoms

    NASA Astrophysics Data System (ADS)

    Singh, S.; Tiwari, V. B.; Kale, Y. B.; Mishra, S. R.; Rawat, H. S.

    2015-09-01

    We report simultaneous cooling and trapping of metastable 84Kr (84Kr*) and metastable 86Kr (86Kr*) atoms by overlapping the cooling laser beams for these different isotopes in the same region of a magneto-optical trap (MOT). Approximately 2 × 105 atoms of each isotope were trapped in this two isotope-MOT (TIMOT). We have investigated the heteronuclear collision trap loss rates for each isotope due to the presence of cold atoms of other isotope using the TIMOT loading curves. The two body heteronuclear loss rate coefficient {β }{84Kr*-{}86Kr*} (i.e. for the loss of 84Kr* due to presence of 86Kr*) and the reciprocal loss rate coefficient {β }{86Kr*-{}84Kr*} (i.e. for the loss of 86Kr* due to presence of 84Kr*) are measured to be (8.7 ± 0.8) × 10-10 cm3 s-1 and (8.8 ± 0.8) × 10-10 cm3 s-1 respectively for laser beam intensity values of 21 mW cm-2 (for cooling of 84Kr*) and 64 mW cm-2 (for cooling of 86Kr*). The dependence of heteronuclear cold collision loss rate on cooling laser beams intensity has also been studied and compared with homonuclear cold collision loss rate.

  2. Single-collision studies of hot atom energy transfer and chemical reaction

    SciTech Connect

    Valentini, J.J. )

    1991-01-01

    This report discusses research in the collision dynamics of translationally hot atoms, with funding with DOE for the project Single-Collision Studies of Hot Atom Energy Transfer and Chemical Reaction,'' Grant Number DE-FG03-85ER13453. The work reported here was done during the period September 9, 1988 through October 31, 1991. During this period this DOE-funded work has been focused on several different efforts: (1) experimental studies of the state-to-state dynamics of the H + RH {yields} H{sub 2} R reactions where RH is CH{sub 4}, C{sub 2}H{sub 6}, or C{sub 3}H{sub 8}, (2) theoretical (quasiclassical trajectory) studies of hot hydrogen atom collision dynamics, (3) the development of photochemical sources of translationally hot molecular free radicals and characterization of the high resolution CARS spectroscopy of molecular free radicals, (4) the implementation of stimulated Raman excitation (SRE) techniques for the preparation of vibrationally state-selected molecular reactants.

  3. Single-collision studies of hot atom energy transfer and chemical reaction. Final report

    SciTech Connect

    Valentini, J.J.

    1991-12-31

    This report discusses research in the collision dynamics of translationally hot atoms, with funding with DOE for the project ``Single-Collision Studies of Hot Atom Energy Transfer and Chemical Reaction,`` Grant Number DE-FG03-85ER13453. The work reported here was done during the period September 9, 1988 through October 31, 1991. During this period this DOE-funded work has been focused on several different efforts: (1) experimental studies of the state-to-state dynamics of the H + RH {yields} H{sub 2} R reactions where RH is CH{sub 4}, C{sub 2}H{sub 6}, or C{sub 3}H{sub 8}, (2) theoretical (quasiclassical trajectory) studies of hot hydrogen atom collision dynamics, (3) the development of photochemical sources of translationally hot molecular free radicals and characterization of the high resolution CARS spectroscopy of molecular free radicals, (4) the implementation of stimulated Raman excitation (SRE) techniques for the preparation of vibrationally state-selected molecular reactants.

  4. Theoretical studies relating to the interaction of radiation with matter: Atomic collision processes occurring in the presence of radiation fields

    NASA Astrophysics Data System (ADS)

    Berman, P. R.

    1983-09-01

    Work is reported in the areas of: Saturation Spectroscopy; Heating and Cooling via Laser-Assisted Collisions; Creation of Electronic State Coherences via Laser-Assisted Collisions; Two-Level Atom Plus Radiation Pulse; Photon as Catalyst; and Collisional Effects in Four-Wave Mixing.

  5. Electronic excitation of ground state atoms by collision with heavy gas particles

    NASA Technical Reports Server (NTRS)

    Hansen, C. Frederick

    1993-01-01

    point where the initial and final potentials cross, or at least come very close. Therefore, this mechanism would be applicable to the case where a gas is initially at very low temperature suddenly subjected to high energy heavy particle bombardment. This situation would model the measurement of excitation cross section by molecular beam techniques, for example. The purpose is to report values of cross sections and rate coefficients for collision excitation of ground state atoms estimated with the Landau-Zener transition theory and to compare results with measurement of excitation cross sections for a beam of Hydrogen atoms impacting Argon atom targets. Some very dubious approximations are used, and the comparison with measurement is found less than ideal, but results are at least consistent within order of magnitude. The same model is then applied to the case of N-N atom collisions, even though the approximations then become even more doubtful. Still the rate coefficients obtained are at least plausible in both magnitude and functional form, and as far as I am aware these are the only estimates available for such rate coefficients.

  6. PREFACE: 8th Asian International Seminar on Atomic and Molecular Physics (AISAMP)

    NASA Astrophysics Data System (ADS)

    Williams, Jim F.; Buckman, Steve; Bieske, Evan J.

    2009-09-01

    These proceedings arose from the 8th Asian International Seminar on Atomic and Molecular Physics (AISAMP) which was held at the University of Western Australia 24-28 November 2008. The history of AISAMP (Takayanagi and Matsuzawa 2002) recognizes its origin from the Japan-China meeting of 1985, and the first use of the name 'The First Asian International Seminar on Atomic and Molecular Physics (AISAMP)' in 1992. The initial attendees, Japan and China, were joined subsequently by scientists from Korea, Taiwan, India, Australia and recently by Malaysia, Thailand, Vietnam, Turkey Iran, UK and USA. The main purpose of the biennial AISAMP series is to create a wide forum for exchanging ideas and information among atomic and molecular scientists and to promote international collaboration. The scope of the AISAMP8 meeting included pure, strategic and applied research involving atomic and molecular structure and processes in all forms of matter and antimatter. For 2008 the AISAMP conference incorporated the Australian Atomic and Molecular Physics and Quantum Chemistry meeting. The topics for AISAMP8 embraced themes from earlier AISAMP meetings and reflected new interests, in atomic and molecular structures, spectroscopy and collisions; atomic and molecular physics with laser or synchrotron radiation; quantum information processing using atoms and molecules; atoms and molecules in surface physics, nanotechnology, biophysics, atmospheric physics and other interdisciplinary studies. The implementation of the AISAMP themes, as well as the international representation of research interests, is indicated both in the contents list of these published manuscripts as well as in the program for the meeting. Altogether, 184 presentations were made at the 8th AISAMP, including Invited Talks and Contributed Poster Presentations, of which 60 appear in the present Proceedings after review by expert referees in accordance with the usual practice of Journal of Physics: Conference Series of

  7. Atomic collisions in suprafluid helium-nanodroplets: timescales for metal-cluster formation derived from He-density functional theory

    PubMed Central

    Volk, Alexander; Thaler, Philipp

    2015-01-01

    Collision times for the coinage metal atoms Cu, Ag and Au in He-droplets are derived from helium density functional theory and molecular dynamics simulations. The strength of the attractive interaction between the metal atoms turns out to be less important than the mass of the propagating metal atoms. Even for small droplets consisting of a few thousand helium atoms, the collision times are shortest for Cu, followed by Ag and Au, despite the higher binding energy of Au2 compared to Cu2. PMID:25812719

  8. The physics of spin polarized atomic vapors

    NASA Astrophysics Data System (ADS)

    Happer, William

    1988-05-01

    Research efforts are focussed on the study of spin polarized atoms, nuclei and electrons during the period covered by this report. Although this work is 6.1 basic research, it has applications to a number of important Air Force problems. For example, the atomic clocks used on the GPS satellite system operate with optically pumped rubidium absorption cells, very similar to the ones being investigated here. A number of the scientists and engineers working on atomic clocks used by Air Force satellite systems were trained with the support of this grant. We have participated in recent Air Force advisory panels to review concepts for high-energy-density fuels based on spin polarized atoms and molecules. The insights gained from research sponsored by this grant have been very useful in evaluating these ideas. Recent work has focussed on two main areas, the investigation of quadrupolar interactions between spin polarized noble gas nuclei and surfaces and the quantitative investigation of how magnetic field inhomogeneities cause spin relaxation.

  9. ATOMIC PHYSICS, AN AUTOINSTRUCTIONAL PROGRAM, VOLUME 2, SUPPLEMENT.

    ERIC Educational Resources Information Center

    DETERLINE, WILLIAM A.; KLAUS, DAVID J.

    THE AUTOINSTRUCTIONAL MATERIALS IN THIS TEXT WERE PREPARED FOR USE IN AN EXPERIMENTAL STUDY, OFFERING SELF-TUTORING MATERIAL FOR LEARNING ATOMIC PHYSICS. THE TOPICS COVERED ARE (1) ISOTOPES AND MASS NUMBERS, (2) MEASURING ATOMIC MASS, (3) DISCOVERY OF THE NUCLEUS, (4) STRUCTURE OF THE NUCLEUS, (5) DISCOVERY OF THE NEUTRON, (6) NUCLEAR REACTIONS,…

  10. Project Physics Tests 5, Models of the Atom.

    ERIC Educational Resources Information Center

    Harvard Univ., Cambridge, MA. Harvard Project Physics.

    Test items relating to Project Physics Unit 5 are presented in this booklet. Included are 70 multiple-choice and 23 problem-and-essay questions. Concepts of atomic model are examined on aspects of relativistic corrections, electron emission, photoelectric effects, Compton effect, quantum theories, electrolysis experiments, atomic number and mass,…

  11. Will Allis Prize for the Study of Ionized Gases Lecture: Electron and Photon Collisions with Atoms and Molecules

    NASA Astrophysics Data System (ADS)

    Burke, Philip G.

    2012-06-01

    After a brief historical introduction this talk will review the broad range of collision processes involving electron and photon collisions with atoms and molecules that are now being considered. Their application in the analysis of astronomical spectra, atmospheric observations and laboratory plasmas will be considered. The talk will review the R-matrix computational method which has been widely used by international collaborations and by other scientists in the field to obtain accurate scattering amplitudes and cross sections of importance in these applications. Results of some recent calculations of electron and photon collisions with atoms and molecules will be presented. In conclusion some challenges for future research will be briefly discussed.

  12. NASA GSFC Science Symposium on Atomic and Molecular Physics

    NASA Technical Reports Server (NTRS)

    Bhatia, Anand K. (Editor)

    2007-01-01

    This document is the proceedings of a conference on atomic and molecular physics in honor of the retirements of Dr. Aaron Temkin and Dr. Richard Drachman. The conference contained discussions on electron, positron, atomic, and positronium physics, as well as a discussion on muon catalyzed fusion. This proceedings document also contains photographs taken at the symposium, as well as speeches and a short biography made in tribute to the retirees.

  13. Physical meaning of the multiplicities of emitted nucleons in hadron-nucleus collisions

    NASA Technical Reports Server (NTRS)

    Strugalski, Z.

    1985-01-01

    The analysis of experimental data on hadron-nucleus collisions at energies from about 2 up to about 400 GeV was performed in order to discover a physical meaning of the multiplicity of emitted nucleons. Simple relations between the multiplicities and the thickness of the nuclear matter layer involved in collisions were obtained.

  14. Effect of electron-nuclei interaction on internuclear motions in slow ion-atom collisions

    NASA Astrophysics Data System (ADS)

    Tolstikhina, Inga Yu.; Tolstikhin, Oleg I.

    2015-10-01

    The electron-nuclei interaction affects the internuclear motion in slow ion-atom collisions, which in turn affects theoretical results for the cross sections of various collision processes. The results are especially sensitive to the details of the internuclear dynamics in the presence of a strong isotope effect on the cross sections, as is the case, e.g., for the charge transfer in low-energy collisions of He2+ with H, D, and T. By considering this system as an example, we show that internuclear trajectories defined by the Born-Oppenheimer (BO) potential in the entrance collision channel, which effectively accounts for the electron-nuclei interaction, are in much better agreement with trajectories obtained in the ab initio electron-nuclear dynamics approach [R. Cabrera-Trujillo et al., Phys. Rev. A 83, 012715 (2011), 10.1103/PhysRevA.83.012715] than the corresponding Coulomb trajectories. We also show that the use of the BO trajectory instead of the Coulomb trajectory in the calculations of the charge-transfer cross sections within the adiabatic approach improves the agreement of the results with ab initio calculations.

  15. Selected bibliography on atomic collisions: Data collections, bibliographies, review articles, books, and papers of particular tutorial value

    SciTech Connect

    McDaniel, E.W.; Flannery, M.R.; Thomas, E.W.; Manson, S.T.

    1985-07-01

    This bibliography deals mainly with binary and ternary collisions involving electrons, photons, and heavy particles (i.e., atoms, molecules, and ions). The energy range covered for each kind of collision is such that the interactions might be described as electronic, atomic, or chemical--higher-energy collisions involving nuclear forces are not treated. Also covered are particle and photon impact on surfaces, the passage of particles and radiation through bulk matter, and transport phenomena in gases. Practically all of the references cited are data compilations, other bibliographies, review articles, or books. The main objective is to provide easy access to atomic collision data, although some references are included principally for their tutorial value.

  16. New results in atomic physics at the Advanced Light Source

    SciTech Connect

    Schlachter, A.S.

    1995-01-01

    The Advanced Light Source is the world's first low-energy third-generation synchrotron radiation source. It has been running reliably and exceeding design specifications since it began operation in October 1993. It is available to a wide community of researchers in many scientific fields, including atomic and molecular science and chemistry. Here, new results in atomic physics at the Advanced Light Source demonstrate the opportunities available in atomic and molecular physics at this synchrotron light source. The unprecedented brightness allows experiments with high flux, high spectral resolution, and nearly 100% linear polarization.

  17. Capture of negative muons by hydrogen atoms at low collision energies

    SciTech Connect

    Sakimoto, Kazuhiro

    2010-01-15

    A rigorous quantum mechanical calculation is carried out for negative muon capture by atomic hydrogen (mu{sup -}+H->mu{sup -}p+e) by using the R-matrix method. The total and final-state selected capture cross sections are calculated at low collision energies ranging from 0.001 to 1 eV. The total capture cross section can, on average, be explained in terms of a previously obtained empirical formula [K. Sakimoto, Phys. Rev. A 66, 032506 (2002)]. However, the present result exhibits additional undulation and cusp structures, which stem from quantum phenomena. The muons are predominantly captured into the highest energetically possible state of mu{sup -}p in the present energy region. However, the mu{sup -}p products having high angular momenta cannot be formed unless the collision energy becomes high.

  18. Rotational excitation of linear molecules by collisions with atoms - Comparison of classical and quantum methods

    NASA Technical Reports Server (NTRS)

    Chapman, S.; Green, S.

    1977-01-01

    Exact quantum results for the rotational excitation of rigid linear molecules by collisions with atoms are compared with classical trajectory results. The systems studied are CO-He, CS-H2, OCS-H2, HCl-He, and HCl-Ar at collision energies up to 500/cm. Total cross sections and state to state rate constants are compared. The classical results are found to be in good agreement with the quantum results on the average. Differences arising from the existence of purely quantum effects are clearly evident, but consistent and predictable. Two methods of extracting state selective information from moments of the classical distribution are examined and found to be less reliable than the usual histogram method. In conjunction with previous comparisons of classical and quantum results these calculations provide a useful measure of the limitations and reliability of classical trajectories.

  19. Reactive collisions of atomic antihydrogen with the H2 and H2+ molecules

    NASA Astrophysics Data System (ADS)

    Cohen, James S.

    2006-09-01

    The fermion molecular dynamics (FMD) method is used to determine the protonium (Pn) formation and total destruction cross sections for collisions of antihydrogen (\\bar{H}) with the H2 molecule and the H2+ molecular ion at collision energies above 0.1 au in the centre-of-mass system. The cross sections and initial quantum numbers are compared with the analogous cross sections for \\bar{H}+H, \\barp+H, \\barp+H_2 and \\barp+H_2^+ previously calculated. Like the \\barp projectile, the protonium-formation cross sections for the \\bar{H} projectile are much larger and extend to higher energies with the molecular targets than with the atomic target. The possibility is considered that a relatively long-lived state of the \\bar{H}H molecule may be formed in rearrangement scattering of \\bar{H}+H_2 at low energies.

  20. Coincidence measurements of electron capture and loss in ion-atom collisions

    SciTech Connect

    DuBois, R.D.

    1990-09-01

    Collisions between fast, fully stripped projectiles and atomic targets predominantly result in target electrons being ejected to the continuum. For fast partially stripped projectiles which bring weakly bound electrons into the collision, projectile ionization can also contribute to the observed electron spectra. At lower impact velocities, electron capture by the projectile ion becomes important and higher order processes, often referred to as transfer ionization, can be a significant source of free electrons. In recent years, coincidence techniques have been used to evaluate the relative importance of electron capture and loss in free electron production, to separate the capture and loss contributions from those resulting from target ionization alone, and to provide more detailed information about electron capture and loss mechanisms than is available from total cross section measurements. A brief survey of these experiments will be presented. 23 refs., 9 figs.

  1. US-Japan workshop on atomic collisions in solids: Abstracts of lectures

    SciTech Connect

    Not Available

    1990-03-01

    This report contains abstracts on the following topics: techniques of scanning probe microscopy; new types of radiation; a search for wake-riding electrons using slow antiproton beams; antiproton wake: theory; bending of swift ion beams by graphite foils; angular momentum distribution of autoionizing rydberg states: produced by 64 MeV S ions in collisions with C foils; multiphonon energy exchange in atom-surface collisions; plans for positron experiments; resonant coherent excitation: experiment; line shapes in resonant coherent excitation: theory; MUSE experiments and Monte Carlo simulation; inelastic interactions of electrons and positrons with solids; density fluctuation detection; cluster-impact fusion; a model for cluster-impact fusion; thoughts on cold fusion; and plasmon decay.

  2. Alkali--rare gas photodissociation lasers: Applications to laser physics and atom-atom interactions

    NASA Astrophysics Data System (ADS)

    Hewitt, John Darby

    This dissertation describes several experiments in which alkali--rare gas laser systems are utilized as a simple platform with which to isolate and study atom-atom interactions and fundamental physical processes that are ill-understood or have never been investigated previously. Specifically, the minimum allowable energy separation between levels 2 and 3 in a three-level laser system has been investigated experimentally, as have two-photon absorption processes in atomic Rb and Cs.

  3. SOHO: Atomic physics and the solar atmosphere

    SciTech Connect

    Kucera, T. A.

    1998-09-28

    Many aspects of the Sun's corona and wind are studied using data from the ultraviolet spectrum. Accurate atomic parameters are needed to interpret these data correctly, and a good understanding of the behaviors of atoms and ions in plasmas is essential to modeling the Sun's atmosphere. Here I present two examples of studies being carried out using the Solar and Heliospheric Observatory (SOHO) extreme ultraviolet spectrographs. The first of these is the study of flows in the Sun's chromosphere and corona. SOHO has provided new information concerning previous observations of the predominant down-flows in the Sun's lower atmosphere. Accurate measurements of Doppler line shifts have been extended to the corona. It has also been found that the Doppler shifts vary over different parts of the Sun. The second study discussed involves the use of SOHO data to measure elemental abundances in coronal structures know as streamers, giving more information on the 'FIP' effect--the observation that there is a relative deficit of elements with high first ionization potentials (FIPs) in the corona and solar wind.

  4. Atomic physics with highly charged ions

    NASA Astrophysics Data System (ADS)

    Richard, P.

    1993-10-01

    The past year has been a busy one for all three accelerators: the LINAC, EBIS, and the tandem. The EBIS continues to deliver beams of highly charged ions around the clock for the study of low energy collisions with gases and surfaces. The electron beam energy was upgraded to 10 keV, and intensities of highly charged species such as Xe(44+) were greatly increased. The tandem, the traditional source of highly charged binary encounter electron production at zero degrees were studied for medium Z (Si,Cl,Cu) projectiles. Recoil momentum spectroscopy has been used to separate the contributions to collisional ionization of one-electron ions (C(5+), O(7+), F(8+)) from the nucleus and the electrons of a He target. Marked structure in the binary encounter electron spectra for Cu(sup q+) on H2 targets was measured for moderate velocity projectiles. Electron capture by slow multiply charged (EBIS) projectiles from laser excited targets has been carried out. Cross sections for capture from Na(3s) and Na*(3p) were measured for velocities between 0.1 and 1 au. The extension of these experiments to laser excited Rydberg targets is proceeding. Electron capture cross sections and average Q values for Ar(16+) on He at velocities between 0.23 and 1.67 au were measured. The charge state distribution of the He recoils following large angle scattering of C(4+) and C(6+) ions at 7.5 keV/u has been measured. Cross sections have been measured for up to sextuple capture from C60 (buckminsterfullerene) by highly charged slow projectiles. Coupled channel calculations for double capture from He by slow multicharge ions were carried out.

  5. The impact of short-range forces on high-energy atom collisions in displacement cascades

    NASA Astrophysics Data System (ADS)

    Samolyuk, German; Stoller, Roger; Tamm, Artur; Beland, Laurent; Stocks, G. Malcolm; Caro, Alfredo; Slipchenko4, Lyudmila; Osetskiy, Yury; Aabloo, Alvo; Klintenberg, Mattias; Wang, Yang

    Simulation of primary radiation damage formation in solid materials involves collisions between atoms with a few hundred keV of kinetic energy. As a result, during these collisions, the distance between two colliding atoms can approach 0.05 nm. For such small atomic separations, interatomic potentials significantly underestimate the potential energy. The common practice involves using a screened Coulomb pair potential to describe the high-energy interactions and to smoothly join this to the equilibrium potential. However, there is no standard method for choosing the joining parameters and defect production during cascade evolution has been shown to be sensitive to how the joining is done. We developed a new procedure, which includes the use of ab initio, calculations to determine the pair interactions at intermediate distances, together with systematic criteria for choosing the joining parameters. Results are presented for the case of nickel. Research at the Oak Ridge National Laboratory and Los Alamos National Laboratory sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, ``Center for Energy Dissipation to Defect Evolution''.

  6. Database for inelastic collisions of sodium atoms with electrons, protons, and multiply charged ions

    SciTech Connect

    Igenbergs, K.; Schweinzer, J.; Bray, I.; Bridi, D.; Aumayr, F.

    2008-11-15

    The available experimental and theoretical cross section data for inelastic collision processes of ground (3s) and excited (3p, 4s, 3d, 4p, 5s, 4d, and 4f) state Na atoms with electrons, protons, and multiply charged ions have been collected and critically assessed. In addition to existing data, electron-impact cross sections, for both excitation and ionization, have been calculated using the convergent close-coupling approach. In the case of proton-impact cross section, the database was enlarged by new atomic-orbital close-coupling calculations. Both electron-impact and proton-impact processes include excitation from the ground state and between excited states (n = 3-5). For electron-impact, ionization from all states is also considered. In the case of proton-impact electron loss, cross sections (the sum of ionization and single-electron charge transfer) are given. Well-established analytical formulae used to fit cross sections, published by Wutte et al. and Schweinzer et al. for collisions with lithium atoms, were adapted to sodium. The 'recommended cross sections' for the processes considered have been critically evaluated and fitted using the adapted analytical formulae. For each inelastic process the fit parameters determined are tabulated. We also present the assessed data in graphical form. The criteria for comprehensively evaluating the accuracy of the experimental data, theoretical calculations, and procedures used in determining the recommended cross sections are discussed.

  7. Multichannel quantum-defect theory for ultracold atom-ion collisions

    NASA Astrophysics Data System (ADS)

    Idziaszek, Zbigniew; Simoni, Andrea; Calarco, Tommaso; Julienne, Paul S.

    2011-08-01

    We develop an analytical model for ultracold atom-ion collisions using the multichannel quantum-defect formalism. The model is based on analytical solutions of the r-4 long-range potential and on the application of a frame transformation between asymptotic and molecular bases. This approach allows the description of atom-ion interaction in the ultracold domain in terms of only three parameters: the singlet and triplet scattering lengths, assumed to be independent of the relative motion angular momentum, and the lead dispersion coefficient of the asymptotic potential. We also introduce corrections to the scattering lengths that improve the accuracy of our quantum-defect model for higher-order partial waves, a particularly important result for an accurate description of shape and Feshbach resonances at finite temperature. The theory is applied to the system composed of a 40Ca+ ion and a Na atom, and compared with numerical coupled-channel calculations carried out using ab initio potentials. For this particular system, we investigate the spectrum of bound states, the rate of charge-transfer processes and the collision rates in the presence of magnetic Feshbach resonances at zero and finite temperature.

  8. Scattering of NH3 and ND3 with rare gas atoms at low collision energy.

    PubMed

    Loreau, J; van der Avoird, A

    2015-11-14

    We present a theoretical study of elastic and rotationally inelastic collisions of NH3 and ND3 with rare gas atoms (He, Ne, Ar, Kr, Xe) at low energy. Quantum close-coupling calculations have been performed for energies between 0.001 and 300 cm(-1). We focus on collisions in which NH3 is initially in the upper state of the inversion doublet with j = 1, k = 1, which is the most relevant in an experimental context as it can be trapped electrostatically and Stark-decelerated. We discuss the presence of resonances in the elastic and inelastic cross sections, as well as the trends in the inelastic cross sections along the rare gas series and the differences between NH3 and ND3 as a colliding partner. We also demonstrate the importance of explicitly taking into account the umbrella (inversion) motion of NH3 in order to obtain accurate scattering cross sections at low collision energy. Finally, we investigate the possibility of sympathetic cooling of ammonia using cold or ultracold rare gas atoms. We show that some systems exhibit a large ratio of elastic to inelastic cross sections in the cold regime, which is promising for sympathetic cooling experiments. The close-coupling calculations are based on previously reported ab initio potential energy surfaces for NH3-He and NH3-Ar, as well as on new, four-dimensional, potential energy surfaces for the interaction of ammonia with Ne, Kr, and Xe, which were computed using the coupled-cluster method and large basis sets. We compare the properties of the potential energy surfaces corresponding to the interaction of ammonia with the various rare gas atoms. PMID:26567658

  9. Current Topics in Atomic, Molecular and Optical Physics

    NASA Astrophysics Data System (ADS)

    Sinha, Chandana; Bhattacharyya, Shib Shankar

    Preface -- Ultrafast dynamics of nano and mesoscopic systems driven by asymmetric electromagnetic pulses / A. Matos-Abiague, A. S. Moskalenko and J. Berakdar -- One-dimensional non-linear oscillators as models for atoms and molecules under intense laser fields / A. Wadehra and B. M. Deb -- Experimenting with topological states of Bose-Einstein condensates / C. Raman -- Laser cooling and trapping of Rb atoms / S. Chakraborty ... [et al.] -- Pair-correlation in Bose-Einstein condensate and fermi superfluid of atomic gases / B. Deb -- Properties of trapped Bose gas in the large-gas-parameter regime / A. Banerjee -- A Feynman-Kac path integral study of Rb gas / S. Datta -- Mean field theory for interacting spin-1 bosons on a lattice / R. V. Pai, K. Sheshadri and R. Pandit -- Mixed internal-external state approach for quantum computation with neutral atoms on atom chips / E. Charron ... [et al.] -- Ultrafast pulse shaping developments for quantum computation / S. K. Karthick Kumar and D. Goswami -- Quantum information transfer in atom-photon interactions in a cavity / A. S. Majumdar, N. Nayak and B. Ghosh -- Liouville density evolution in billiards and the quantum connection / D. Biswas -- MRCPA: theory and application to highly correlating system / K. Tanaka -- Calculation of negative ion shape resonances using coupled cluster theory / Y. Sajeev and S. Pal -- Optical frequency standard with Sr+: a theoretical many-body approach / C. Sur ... [et al.] -- Fast heavy ion collisions with H[symbol] molecules and young type interference / L. C. Tribedi and D. Misra -- Estimation of ion kinetic energies from time-of-flight and momentum spectra / B. Bapat -- Third-order optical susceptibility of metal nanocluster-glass 28 composites / B. Ghosh and P. Chakraborty -- Study of atom-surface interaction using magnetic atom mirror / A. K. Mohapatra.

  10. Experimental determination of the real elements of the density matrix of H({ital n}=3) atoms produced in 20--100-keV collisions of H{sup +} on Kr

    SciTech Connect

    Seifert, N.; Gibson, N.D.; Risley, J.S.

    1995-11-01

    In continuation of our previous work, charge transfer processes occurring in protons on rare-gas-atom collisions have been investigated. Diagonal and real off-diagonal coherence elements of the density matrix for H({ital n}=3) atoms produced in 20--100-keV electron-capture collisions with Kr atoms are experimentally determined by analyzing the Balmer-{alpha} light from the decay of H atoms from the ({ital n}=3) state to the ({ital n}=2) state. The intensity and polarization of the emitted light are measured as functions of an axially symmetric electric field in the collision region. These data are fitted to a numerical model of the H atom in an electric field in order to extract density-matrix elements. The results are compared to previous studies of H{sup +} on He and Ar. The collisionally produced dipole moment of the H({ital n}=3) atom decreases for increasing atomic number of the rare-gas target atoms, which indicates that the final phase of the collision process is not essential for the formation of the dipole moment. This physical picture is further supported by our alignment data. Absolute cross sections for charge transfer to the 3{ital s}, 3{ital p}, and 3{ital d} levels are presented as well.

  11. Charge transfer reactions in multiply charged ion-atom collisions. [in interstellar clouds

    NASA Technical Reports Server (NTRS)

    Steigman, G.

    1975-01-01

    Charge-transfer reactions in collisions between highly charged ions and neutral atoms of hydrogen and/or helium may be rapid at thermal energies. If these reactions are rapid, they will suppress highly charged ions in H I regions and guarantee that the observed absorption features from such ions cannot originate in the interstellar gas. A discussion of such charge-transfer reactions is presented and compared with the available experimental data. The possible implications of these reactions for observations of the interstellar medium, H II regions, and planetary nebulae are outlined.

  12. TlII excitation cross-sections in collisions of slow electrons with thallium atoms

    NASA Astrophysics Data System (ADS)

    Smirnov, Yu M.

    2016-09-01

    Excitation of a singly-charged thallium ion in electron collisions with thallium atoms has been studied experimentally. Seventy excitation cross sections have been measured at an exciting electron energy of 30 eV. Ten optical excitation functions (OEFs) have been recorded in the incident electron energy range of 0–200 eV. For seven TlII spectral series, the dependence of excitation cross-sections on the principal quantum numbers of upper levels has been studied. A comparison of findings with data from preceding publications is presented.

  13. Charge-transfer-induced evaporation in collisions of Li2+31 clusters with Cs atoms

    NASA Astrophysics Data System (ADS)

    Bréchignac, C.; Cahuzac, Ph.; Concina, B.; Leygnier, J.; Ruiz, L. F.; Zarour, B.; Hervieux, P. A.; Hanssen, J.; Politis, M. F.; Martín, F.

    2003-12-01

    We present a combined theoretical and experimental study of dissociative charge transfer in collisions of slow Li2+31 clusters with Cs atoms. We provide a direct quantitative comparison between theory and experiment and show that good agreement is only found when the experimental time-of-flight and initial cluster temperature are taken into account in the theoretical modeling. This model explains evaporation as resulting from a collisional energy deposit due to cluster electronic excitation during charge transfer. We discuss in detail the basic mechanisms that are responsible for the charge-transfer reaction and different approximations to evaluate the energy deposit.

  14. Loss and excitation in single collisions of highly-stripped heavy ions with atoms

    SciTech Connect

    Graham, W.G.; Bernstein, E.M.; Clark, M.W.; Oglesby, C.S.; Tanis, J.A.; Berkner, K.H.; Gohil, P.; Schlachter, A.S.; Stearns, J.W.; Johnson, B.M.

    1986-01-01

    Cross sections for projectile loss and excitation (LE) in single collisions of heavy ions with atoms have been measured for 15 to 460 MeV S, Ar, Ca, and V ions, with charge states varying from 12+ to 21+ in H/sub 2/, He, Ne, and Ar gas targets. The results indicate that K x-ray production takes place through excitation rather than loss of a 1s electron. An independent electron model appears to provide a reasonable description of LE for Li-like projectiles. However, there are also indications that loss and excitation events are correlated. 11 refs., 4 figs.

  15. Laboratory studies of atomic collision processes of importance in planetary atmospheres

    NASA Technical Reports Server (NTRS)

    Stebbings, R. F.; Smith, K.

    1984-01-01

    Progress in the following research supported under NSG 7386 is reported: (1) measurement of differential cross sections for atomic and molecular collisions relevant to analysis and modeling of data from Pioneer 11, Pioneer 12, Voyager 1, and Voyager 2; (2) analysis of measured differential cross section results to provide scattering data in forms that are easy to apply to atmospheric modeling work; (3) analysis of the data to give basic information on the molecular potentials involved in the scattering process; and (4) development and initial use of apparatus to study dissociative processes in neutral molecules.

  16. Classical-quantum correspondence for ionization in fast ion-atom collisions

    SciTech Connect

    Burgdoerfer, J. |; Reinhold, C.O.

    1994-10-01

    We analyze the interplay between classical and quantum dynamics in ionization of atoms by fast charged particles The convergence to the classical limit is studied as a function of the momentum transferred to the electron during the collision, the impact parameter. the energy and angle of the emitted electron, and the initial state of the target. One goal is to assess the validity of exact classical (CTMC) methods and approximate classical models such as the Thomson model. Applications to data for electron ejection at large angles are presented. The connection between collisional ionization by charged particles and ionization by half-cycle pulses is discussed.

  17. Rotational excitation of symmetric top molecules by collisions with atoms. II - Infinite order sudden approximation

    NASA Technical Reports Server (NTRS)

    Green, S.

    1979-01-01

    The infinite order sudden (IOS) approximation is extended to rotational excitation of symmetric tops by collisions with atoms. After development of a formalism for 'primitive' or 'one-ended' tops, proper parity-adapted linear combinations describing real rotors are considered and modifications needed for asymmetric rigid rotors are noted. The generalized spectroscopic relaxation cross sections are discussed. IOS calculations for NH3-He and H2CO-He are performed and compared with more accurate calculations, and the IOS approximation is found to provide a reasonably accurate description.

  18. Quantifying the physical demands of collision sports: does microsensor technology measure what it claims to measure?

    PubMed

    Gabbett, Tim J

    2013-08-01

    The physical demands of rugby league, rugby union, and American football are significantly increased through the large number of collisions players are required to perform during match play. Because of the labor-intensive nature of coding collisions from video recordings, manufacturers of wearable microsensor (e.g., global positioning system [GPS]) units have refined the technology to automatically detect collisions, with several sport scientists attempting to use these microsensors to quantify the physical demands of collision sports. However, a question remains over the validity of these microtechnology units to quantify the contact demands of collision sports. Indeed, recent evidence has shown significant differences in the number of "impacts" recorded by microtechnology units (GPSports) and the actual number of collisions coded from video. However, a separate study investigated the validity of a different microtechnology unit (minimaxX; Catapult Sports) that included GPS and triaxial accelerometers, and also a gyroscope and magnetometer, to quantify collisions. Collisions detected by the minimaxX unit were compared with video-based coding of the actual events. No significant differences were detected in the number of mild, moderate, and heavy collisions detected via the minimaxX units and those coded from video recordings of the actual event. Furthermore, a strong correlation (r = 0.96, p < 0.01) was observed between collisions recorded via the minimaxX units and those coded from video recordings of the event. These findings demonstrate that only one commercially available and wearable microtechnology unit (minimaxX) can be considered capable of offering a valid method of quantifying the contact loads that typically occur in collision sports. Until such validation research is completed, sport scientists should be circumspect of the ability of other units to perform similar functions. PMID:23090320

  19. The dependence of scattering length on van der Waals interaction and reduced mass of the system in two-atomic collision at cold energies

    NASA Astrophysics Data System (ADS)

    RAY, HASI

    2016-06-01

    The static-exchange model (SEM) and the modified static-exchange model (MSEM) recently introduced by Ray [1] is applied to study the elastic collision between two hydrogen-like atoms when both are in ground states considering the system as a four-body Coulomb problem in the center of mass frame, in which all the Coulomb interaction terms in direct and exchange channels are treated exactly. The SEM includes the non-adiabatic short-range effect due to electron-exchange. The MSEM added in it, the long-range effect due to induced dynamic dipole polarizabilities between the atoms e.g. the Van der Waals interaction. Applying the SEM code in different H-like two-atomic systems, a reduced mass dependence on scattering length is observed. Again applying the MSEM code on H(1s)-H(1s) elastic scattering and varying the minimum values of interatomic distance, the dependence of scattering length on the effective interatomic potential consistent with the existing physics are observed. Both these basic findings in low and cold energy atomic collision physics are quite useful and are being reported for the first time.

  20. Atoms in Flight: The Remarkable Connections between Atomic and Hadronic Physics

    SciTech Connect

    Brodsky, Stanley J.; /SLAC

    2012-02-16

    Atomic physics and hadron physics are both based on Yang Mills gauge theory; in fact, quantum electrodynamics can be regarded as the zero-color limit of quantum chromodynamics. I review a number of areas where the techniques of atomic physics provide important insight into the theory of hadrons in QCD. For example, the Dirac-Coulomb equation, which predicts the spectroscopy and structure of hydrogenic atoms, has an analog in hadron physics in the form of light-front relativistic equations of motion which give a remarkable first approximation to the spectroscopy, dynamics, and structure of light hadrons. The renormalization scale for the running coupling, which is unambiguously set in QED, leads to a method for setting the renormalization scale in QCD. The production of atoms in flight provides a method for computing the formation of hadrons at the amplitude level. Conversely, many techniques which have been developed for hadron physics, such as scaling laws, evolution equations, and light-front quantization have equal utility for atomic physics, especially in the relativistic domain. I also present a new perspective for understanding the contributions to the cosmological constant from QED and QCD.

  1. The Common Elements of Atomic and Hadronic Physics

    SciTech Connect

    Brodsky, Stanley J.

    2015-02-26

    Atomic physics and hadronic physics are both governed by the Yang Mills gauge theory Lagrangian; in fact, Abelian quantum electrodynamics can be regarded as the zero-color limit of quantum chromodynamics. I review a number of areas where the techniques of atomic physics can provide important insight into hadronic eigenstates in QCD. For example, the Dirac-Coulomb equation, which predicts the spectroscopy and structure of hydrogenic atoms, has an analog in hadron physics in the form of frame-independent light-front relativistic equations of motion consistent with light-front holography which give a remarkable first approximation to the spectroscopy, dynamics, and structure of light hadrons. The production of antihydrogen in flight can provide important insight into the dynamics of hadron production in QCD at the amplitude level. The renormalization scale for the running coupling is unambiguously set in QED; an analogous procedure sets the renormalization scales in QCD, leading to scheme-independent scale-fixed predictions. Conversely, many techniques which have been developed for hadron physics, such as scaling laws, evolution equations, the quark-interchange process and light-front quantization have important applicants for atomic physics and photon science, especially in the relativistic domain.

  2. Spectroscopy and atomic physics of highly ionized Cr, Fe, and Ni for tokamak plasmas

    NASA Technical Reports Server (NTRS)

    Feldman, U.; Doschek, G. A.; Cheng, C.-C.; Bhatia, A. K.

    1980-01-01

    The paper considers the spectroscopy and atomic physics for some highly ionized Cr, Fe, and Ni ions produced in tokamak plasmas. Forbidden and intersystem wavelengths for Cr and Ni ions are extrapolated and interpolated using the known wavelengths for Fe lines identified in solar-flare plasmas. Tables of transition probabilities for the B I, C I, N I, O I, and F I isoelectronic sequences are presented, and collision strengths and transition probabilities for Cr, Fe, and Ni ions of the Be I sequence are given. Similarities of tokamak and solar spectra are discussed, and it is shown how the atomic data presented may be used to determine ion abundances and electron densities in low-density plasmas.

  3. Charge exchange collisions of slow C6 + with atomic and molecular H

    NASA Astrophysics Data System (ADS)

    Saha, Bidhan C.; Guevara, Nicolais L.; Sabin, John R.; Deumens, Erik; Öhrn, Yngve

    2016-04-01

    Charge exchange in collisions of C6+ ions with H and H2 is investigated theoretically at projectile energies 0.1 < E < 10 keV/amu, using electron nuclear dynamics (END) - a semi-classical approximation which not only includes electron translation factors for avoiding spurious couplings but also employs full dynamical trajectories to treat nuclear motions. Both the total and partial cross sections are reported for the collision of C6+ ions with atomic and molecular hydrogen. A comparison with other theoretical and experimental results shows, in general good agreement except at very low energy, considered here. For H2, the one- and two-electron charge exchange cross sections are calculated and compared with other theoretical and experimental results. Small but non-negligible isotope effects are found at the lowest energy studied in the charge transfer of C6+ with H. In low energy region, it is observed that H2 has larger isotope effects than H atom due to the polarizability effect which is larger than the mass effect.

  4. Inner shell contribution to multiple ionization in ion-atom collisions

    SciTech Connect

    DuBois, R.D.; Toburen, L.H.; Manson, S.T.

    1984-08-01

    Energetic proton impact ionization data for atomic targets is useful in testing our theoretical understanding of atomic collisions. In general, our understanding of bare projectile impact leading to single target ionization is quite good. Multiple ionization mechanisms are, however, less well understood. In certain cases, multiple ionization can account for as much as 50% of the total ionization cross section and thus cannot be neglected in modeling the collision process. Multiple target ionization can occur in a variety of ways. In order to fully analyze the collisional process, cross sections for each of these ionization pathways are necessary but, in general, are unavailable. However, in certain cases combining various experimental and theoretical data allows us to obtain some information about channels heretofore unmeasured. Our purpose here is to outline a procedure that we are currently using to unravel the complex multiple ionization process. In some cases, cross sections for specific ionization pathways can be obtained while in others only information about total contributions of specific ionization channels is available.

  5. Wave-packet continuum-discretization approach to ion-atom collisions: Nonrearrangement scattering

    NASA Astrophysics Data System (ADS)

    Abdurakhmanov, I. B.; Kadyrov, A. S.; Bray, I.

    2016-08-01

    A general single-center close-coupling approach based on a continuum-discretization procedure is developed to calculate excitation and ionization processes in ion-atom collisions. The continuous spectrum of the target is discretized using stationary wave packets constructed from the Coulomb wave functions, the eigenstates of the target Hamiltonian. Such continuum discretization allows one to generate pseudostates with arbitrary energies and distribution. These features are ideal for detailed differential ionization studies. The approach starts from the semiclassical three-body Schrödinger equation for the scattering wave function and leads to a set of coupled differential equations for the transition probability amplitudes. To demonstrate its utility the method is applied to calculate collisions of antiprotons with atomic hydrogen. A comprehensive set of benchmark results from integrated to fully differential cross sections for antiproton-impact ionization of hydrogen in the energy range from 1 keV to 1 MeV is provided. Contrary to previous predictions, we find that at low incident energies the singly differential cross section has a maximum away from the zero emission energy. This feature could not be seen without a fine discretization of the low-energy part of the continuum.

  6. Ionization at the Noble Gases Ion-Atom Collisions in the 1-7 KeV Energy Range

    NASA Astrophysics Data System (ADS)

    Kikiani, Boris; Chitaladze, Marika; Japaridze, Josif; Kavlashvili, Nana

    2002-10-01

    The absolute total cross sections for production of free electrons, all positive show target gas ions and partial cross sections for production of double charged slow target gas ions at these collisions have been measured. The measurements were carried out by improved transfers electric field ("condenser") and magnetic mass-analyzer methods[1]. It was shown that in the investigated energy range practically there are now slow ions with charged state more than two. Control experiments have been shown that process of electron's liberation from fast particles ("stripping" process) is unlikely in the investigated energy range. Therefore, one can to suppose that total cross sections for productions of free electrons are equal to the total cross sections of ionization of the target gas atoms. For symmetrical pairs of colliding particles (He+ _ He, Ne+ _ Ne , etc) and for pairs He+ _ Ne, Ar+ _ Kr and Kr+ _ Xe values of partial cross-sections are negligible. In the cases of He+ _ Kr and He+ _ Xe pairs value of these partial cross sections increases with colliding energy and reaches about three percent at the energy 4kev. However, in the cases of He+ _ Ar, Na+ _ Ar, Kr, Xe the values of relative portion of the double charged ions in the total amount of slow positive ions are significant (for example in He+ _ Ar collision at the energy of 4kev this portion is about 20-25 percent). Analyzes of the correlation diagrams of the diabetics terms of colliding particles system (MS) [2] show that the electron capture processes are accompanying by simultaneous excitation of auto- ionization states of target gas ions. The decay of these states are responsible for realize of double ionization process of the target gas atoms. 1. B. Kikiani, R.Lomsadze, N. Mosulishvili, Proceedings of Tbilisi State University, Physics, 34, 114, 1999; 2 M. Barat, W.Lichten, Phys. Rev, A6, 211, 1972.

  7. Forward electron production in heavy ion-atom and ion-solid collisions

    SciTech Connect

    Sellin, I.A.

    1984-01-01

    A sharp cusp in the velocity spectrum of electrons, ejected in ion-atom and ion-solid collisions, is observed when the ejected electron velocity vector v/sub e/ matches that of the emergent ion vector v/sub p/ in both speed and direction. In ion-atom collisions, the electrons originate from capture to low-lying, projectile-centered continuum states (ECC) for fast bare or nearly bare projectiles, and from loss to those low-lying continuum states (ELC) when loosely bound projectile electrons are available. Most investigators now agree that ECC cusps are strongly skewed toward lower velocities, and exhibit full widths half maxima roughly proportional to v/sub p/ (neglecting target-shell effects, which are sometimes strong). A close examination of recent ELC data shows that ELC cusps are instead nearly symmetric, with widths nearly independent on v/sub p/ in the velocity range 6 to 18 a.u., a result only recently predicted by theory. Convoy electron cusps produced in heavy ion-solid collisions at MeV/u energies exhibit approximately velocity-independent widths very similar to ELC cusp widths. While the shape of the convoy peaks is approximately independent of projectile Z, velocity, and of target material, it is found that the yields in polycrystalline targets exhibit a strong dependence on projectile Z and velocity. While attempts have been made to link convoy electron production to binary ECC or ELC processes, sometimes at the last layer, or alternatively to a solid-state wake-riding model, our measured dependences of cusp shape and yield on projectile charge state and energy are inconsistent with the predictions of available theories. 10 references, 8 figures, 1 table.

  8. A Investigation of a Possible Molecular Effect in Ion Atom Collision Using a Gaseous Argon Target

    NASA Astrophysics Data System (ADS)

    Arora, Sanjeev

    1992-01-01

    The present work deals with an investigation of the molecular effect, which is defined as the difference in experimental results using isotachic atomic ion and molecular ion beams in ion atom collisions. Previous studies have dealt almost exclusively with total cross section measurements. This thesis explores the idea that the molecular effect may be more pronounced in the differential ionization probability of the target atoms. Also, a gaseous argon target of sufficiently low density was used in order to ensure that the two correlated protons in the H _2^{+} beam did not interact with two adjacent target atoms simultaneously. We report that, contrary to the expectations noted above, the molecular effect in the K shell differential ionization probability of argon for scattering angles up to 90^circ appears to be no more than the molecular effect in the total ionization probability. The uncertainity in our results is statistical in nature and can be improved upon by running the experiment for a longer duration of time.

  9. Zeeman relaxation of cold atomic iron and nickel in collisions with {sup 3}He

    SciTech Connect

    Johnson, Cort; Newman, Bonna; Kleppner, Daniel; Greytak, Thomas J.; Brahms, Nathan; Doyle, John M.

    2010-06-15

    We have measured the ratio {gamma} of the diffusion cross section to the angular momentum reorientation cross section in the colliding Fe-{sup 3}He and Ni-{sup 3}He systems. Nickel (Ni) and iron (Fe) atoms are introduced via laser ablation into a cryogenically cooled experimental cell containing cold (<1 K) {sup 3}He buffer gas. Elastic collisions rapidly cool the translational temperature of the ablated atoms to the {sup 3}He temperature. {gamma} is extracted by measuring the decays of the atomic Zeeman sublevels. For our experimental conditions, thermal energy is comparable to the Zeeman splitting. As a result, thermal excitations between Zeeman sublevels significantly impact the observed decay. To determine {gamma} accurately, we introduce a model of Zeeman-state dynamics that includes thermal excitations. We find {gamma}{sub Ni-}{sup 3}{sub He}=5x10{sup 3} and {gamma}{sub Fe-}{sup 3}{sub He{<=}}3x10{sup 3} at 0.75 K in a 0.8-T magnetic field. These measurements are interpreted in the context of submerged shell suppression of spin relaxation, as studied previously in transition metals and rare-earth-metal atoms [C. I. Hancox, S. C. Doret, M. T. Hummon, R. V. Krems, and J. M. Doyle, Phys. Rev. Lett. 94, 013201 (2005); C. I. Hancox, S. C. Doret, M. T. Hummon, L. Luo, and J. M. Doyle, Nature (London) 431, 281 (2004); A. Buchachenko, G. Chaasiski, and M. Szczniak, Eur. Phys. J. D 45, 147 (2007)].

  10. A molecular dynamics simulation of hydrogen atoms collisions on an H-preadsorbed silica surface

    NASA Astrophysics Data System (ADS)

    Rutigliano, M.; Gamallo, P.; Sayós, R.; Orlandini, S.; Cacciatore, M.

    2014-08-01

    The interaction of hydrogen atoms and molecules with a silica surface is relevant for many research and technological areas. Here, the dynamics of hydrogen atoms colliding with an H-preadsorbed β-cristobalite (0 0 1) surface has been studied using a semiclassical collisional method in conjunction with a recently developed analytical potential energy surface based on density functional theory (DFT) calculations. The atomic recombination probability via an Eley-Rideal (E-R) mechanism, as well as the probabilities for other competitive surface processes, have been determined in a broad range of collision energies (0.04-3.0 eV) for off-normal (θv = 45°) and normal (θv = 0°) incidence and for two different surface temperatures (TS = 300 and 1000 K). H2,gas molecules form in roto-vibrational excited levels while the energy transferred to the solid surface is below 10% for all simulated conditions. Finally, the global atomic recombination coefficient (γE-R) and vibrational state resolved recombination coefficients (γ(v)) were calculated and compared with the available experimental values. The calculated collisional data are of interest in chemical kinetics studies and fluid dynamics simulations of silica surface processes in H-based low-temperature, low-pressure plasmas.

  11. Feshbach resonances and transition rates for cold homonuclear collisions between {sup 39}K and {sup 41}K atoms

    SciTech Connect

    Lysebo, M.; Veseth, L.

    2010-03-15

    We report results from close-coupling calculations for homonuclear ultracold collisions between potassium atoms, using the most up-to-date Born-Oppenheimer potential curves. The present study includes both of the bosonic isotopes {sup 39}K and {sup 41}K. The s-wave scattering lengths as functions of the magnetic field strength for collisions between atoms in identical and different hyperfine states are obtained. Several Feshbach resonances are located and characterized for both isotopes. Comparison with experiments, where such data are available, show excellent agreement. We also study weakly bound molecular states of the K{sub 2} molecule in close relation to the calculated Feshbach resonances. Another objective of the present work is to study inelastic collisions in which the hyperfine states of the colliding atoms are changed. From this type of calculation we obtain transition rates as functions of the magnetic field strength. Finally, we discuss how such transition rates might be of importance for experimental work.

  12. Majorana: From Atomic and Molecular, to Nuclear Physics

    NASA Astrophysics Data System (ADS)

    Pucci, R.; Angilella, G. G. N.

    2006-10-01

    In the centennial of Ettore Majorana's birth (1906-1938?), we re-examine some aspects of his fundamental scientific production in atomic and molecular physics, including a not well known short communication. There, Majorana critically discusses Fermi's solution of the celebrated Thomas-Fermi equation for electron screening in atoms and positive ions. We argue that some of Majorana's seminal contributions in molecular physics already prelude to the idea of exchange interactions (or Heisenberg-Majorana forces) in his later workson theoretical nuclear physics. In all his papers, he tended to emphasize the symmetries at the basis of a physical problem, as well as the limitations, rather than the advantages, of the approximations of the method employed.

  13. Near-threshold photoionization of hydrogenlike uranium studied in ion-atom collisions via the time-reversed process.

    PubMed

    Stöhlker, T; Ma, X; Ludziejewski, T; Beyer, H F; Bosch, F; Brinzanescu, O; Dunford, R W; Eichler, J; Hagmann, S; Ichihara, A; Kozhuharov, C; Krämer, A; Liesen, D; Mokler, P H; Stachura, Z; Swiat, P; Warczak, A

    2001-02-01

    Radiative electron capture, the time-reversed photoionization process occurring in ion-atom collisions, provides presently the only access to photoionization studies for very highly charged ions. By applying the deceleration mode of the ESR storage ring, we studied this process in low-energy collisions of bare uranium ions with low- Z target atoms. This technique allows us to extend the current information about photoionization to much lower energies than those accessible for neutral heavy elements in the direct reaction channel. The results prove that for high- Z systems, higher-order multipole contributions and magnetic corrections persist even at energies close to the threshold. PMID:11177990

  14. HISTRAP proposal: heavy ion storage ring for atomic physics

    SciTech Connect

    Olsen, D.K.; Alton, G.D.; Datz, S.; Dittner, P.F.; Dowling, D.T.; Haynes, D.L.; Hudson, E.D.; Johnson, J.W.; Lee, I.Y.; Lord, R.S.

    1986-11-01

    HISTRAP, Heavy Ion Storage Ring for Atomic Physics, is a proposed 46.8-m-circumference synchrotron-cooling-storage ring optimized to accelerate, decelerate, and store beams of highly charged very-heavy ions at energies appropriate for advanced atomic physics research. The ring is designed to allow studies of electron-ion, photon-ion, ion-atom, and ion-ion interactions. An electron cooling system will provide ion beams with small angular divergence and energy spread for precision spectroscopic studies and also is necessary to allow the deceleration of heavy ions to low energies. HISTRAP will have a maximum bending power of 2.0 Tm and will be injected with ions from either the existing Holifield Heavy Ion Research Facility 25-MV tandem accelerator or from a dedicated ECR source and 250 keV/nucleon RFQ linac.

  15. Excitation and charge transfer in low-energy hydrogen-atom collisions with neutral atoms: Theory, comparisons, and application to Ca

    NASA Astrophysics Data System (ADS)

    Barklem, Paul S.

    2016-04-01

    A theoretical method is presented for the estimation of cross sections and rates for excitation and charge-transfer processes in low-energy hydrogen-atom collisions with neutral atoms, based on an asymptotic two-electron model of ionic-covalent interactions in the neutral atom-hydrogen-atom system. The calculation of potentials and nonadiabatic radial couplings using the method is demonstrated. The potentials are used together with the multichannel Landau-Zener model to calculate cross sections and rate coefficients. The main feature of the method is that it employs asymptotically exact atomic wave functions, which can be determined from known atomic parameters. The method is applied to Li+H , Na+H , and Mg+H collisions, and the results compare well with existing detailed full-quantum calculations. The method is applied to the astrophysically important problem of Ca+H collisions, and rate coefficients are calculated for temperatures in the range 1000-20 000 K.

  16. Bringing atomic and nuclear physics laboratory data into the classroom

    SciTech Connect

    Norman, Eric B.; Larimer, Ruth-Mary; Rech, Gregory; Lee, Jeffrey; Vue, Chue; Leubane, Tholoana; Zamvil, Kenneth; Guthrie, Laura

    2003-05-27

    To illustrate a number of basic concepts in atomic and nuclear physics, we have developed three websites where students can analyze data from modern laboratories. By working through the on-line procedures, students will become acquainted with characteristic x-ray spectra, the concept of half-life, x-ray fluorescence, and neutron activation analysis.

  17. Project Physics Reader 5, Models of the Atom.

    ERIC Educational Resources Information Center

    Harvard Univ., Cambridge, MA. Harvard Project Physics.

    As a supplement to Project Physics Unit 5, a collection of articles is presented in this reader for student browsing. Nine excerpts are given under the following headings: failure and success, Einstein, Mr. Tompkins and simultaneity, parable of the surveyors, outside and inside the elevator, the teacher and the Bohr theory of atom, Dirac and Born,…

  18. ATOMIC PHYSICS, AN AUTOINSTRUCTIONAL PROGRAM, VOLUME 4, SUPPLEMENT.

    ERIC Educational Resources Information Center

    DETERLINE, WILLIAM A.; KLAUS, DAVID J.

    THE AUTOINSTRUCTIONAL MATERIALS IN THIS TEXT WERE PREPARED FOR USE IN AN EXPERIMENTAL STUDY, OFFERING SELF-TUTORING MATERIAL FOR LEARNING ATOMIC PHYSICS. THE TOPICS COVERED ARE (1) RADIATION USES AND NUCLEAR FISSION, (2) NUCLEAR REACTORS, (3) ENERGY FROM NUCLEAR REACTORS, (4) NUCLEAR EXPLOSIONS AND FUSION, (5) A COMPREHENSIVE REVIEW, AND (6) A…

  19. ATOMIC PHYSICS, AN AUTOINSTRUCTIONAL PROGRAM, VOLUME 3, SUPPLEMENT.

    ERIC Educational Resources Information Center

    DETERLINE, WILLIAM A.; KLAUS, DAVID J.

    THE AUTOINSTRUCTIONAL MATERIALS IN THIS TEXT WERE PREPARED FOR USE IN AN EXPERIMENTAL STUDY, OFFERING SELF-TUTORING MATERIAL FOR LEARNING ATOMIC PHYSICS. THE TOPICS COVERED ARE (1) NUCLEAR BINDING ENERGY, (2) DISCOVERY OF RADIOACTIVITY, (3) RADIOACTIVE RADIATIONS, (4) ALPHA AND BETA DECAY, (5) BETA DECAY REACTIONS, (6) RADIOACTIVE DATING AND…

  20. Interaction of positronium with helium atoms — the classical treatment of the 5-body collision system

    NASA Astrophysics Data System (ADS)

    Tőkési, Károly; DuBois, Robert D.; Mukoyama, Takeshi

    2014-09-01

    The interaction between positronium and a helium atom is studied using the 5-body classical trajectory Monte Carlo method. We present the total cross sections for the dominant channels, namely for single ionization of the target, and ionization of the projectile, resulting from pure ionization and also from electron transfer (capture or loss) processes for 1-5.7 a.u. incident velocities of the positronium atom. Our results were compared with the calculated data using hydrogen projectiles having the same velocities as well as with the experimental data in collisions between H and He [R.D. DuBois, Á. Kövér, Phys. Rev. A 40, 3605 (1989)]. We analyze the similarities and deviations for ionization of helium atoms by positronium and hydrogen projectile impact. Contribution to the Topical Issue "Electron and Positron Induced Processes", edited by Michael Brunger, Radu Campeanu, Masamitsu Hoshino, Oddur Ingólfsson, Paulo Limão-Vieira, Nigel Mason, Yasuyuki Nagashima and Hajime Tanuma.

  1. Treasure of the Past X: A Spectroscopic Determination of Scattering Lengths for Sodium Atom Collisions

    PubMed Central

    Tiesinga, Eite; Williams, Carl J.; Julienne, Paul S.; Jones, Kevin M.; Lett, Paul D.; Phillips, William D.

    2002-01-01

    We report a preliminary value for the zero magnetic field Na 2S(f = 1, m = − 1) + Na 2S(f = 1, m = − 1) scattering length, a1,−1. This parameter describes the low-energy elastic two-body processes in a dilute gas of composite bosons and determines, to a large extent, the macroscopic wavefunction of a Bose condensate in a trap. Our scattering length is obtained from photoassociative spectroscopy with samples of uncondensed atoms. The temperature of the atoms is sufficiently low that contributions from the three lowest partial waves dominate the spectrum. The observed lineshapes for the purely long-range 0g− molecular state enable us to establish key features of the ground state scattering wavefunction. The fortuitous occurrence of a p-wave node near the deepest point (Re = 72 a0) of the 0g− potential curve is instrumental in determining a1,−1 = (52 ± 5) a0 and a2.2 = (85 ± 3) a0, where the latter is for a collision of two Na 2S(f = 2, m = 2) atoms.

  2. Rovibrationally Inelastic Atom-Molecule Collision Cross Sections from a Hard Sphere Model

    NASA Astrophysics Data System (ADS)

    Lashner, Jacob; Stewart, Brian

    2016-05-01

    Hard-shell models have long been used to elucidate the principal features of molecular energy transfer and exchange reaction in the A + BC system. Nevertheless, no three-dimensional hard-shell calculation of inelastic collision cross sections has been reported. This work aims to fill that void. A particular motivation comes from our experimental results, which show the importance of equatorial impacts in the vibrational excitation process. Working with the simple hard-sphere model, we incorporated secondary impacts, defined as those in which A strikes C after striking B. Such collisions are important in systems such as Li2 - X, in which vibrational energy transfer occurs principally through side impacts. We discuss the complexity this adds to the model and present fully three-dimensional cross sections for rovibrational excitation of an initially stationary molecule in the homonuclear A + B2 system, examining the cross section as a function of the masses and radii of the atoms. We show how the features in the cross section evolve as these parameters are varied and calculate the contribution of secondary (near-equatorial) impacts to the dynamics. We compare with recent measurements in our laboratory and with the results of quasiclassical trajectories.

  3. Atomic physics of strongly correlated systems. Progress report, 1 August 1980-31 July 1981

    SciTech Connect

    Lin, C.D.

    1981-03-01

    Studies of electron correlations of doubly-excited electrons in hyperspherical coordinates, and differential and total cross sections for charge transfer and ionization in fast ion-atom collisions are reported. (GHT)

  4. B physics at CDF - the Beauty of hadron collisions

    SciTech Connect

    Tonelli, Diego

    2010-11-01

    The CDF experiment at the Tevatron p{bar p} collider established that extensive and detailed exploration of the b-quark dynamics is possible in hadron collisions, with results competitive and supplementary to those from e{sup +}e{sup -} colliders. This provides an unique, rich, and highly rewarding program that is currently reaching full maturity. I report a few recent world-leading results on rare decays, CP-violation in B{sub s}{sup 0} mixing, and b {yields} s penguin decays.

  5. Redistribution - Why half a collision is better than a whole one. [spectra of scattered light from perturbed atomic system

    NASA Technical Reports Server (NTRS)

    Cooper, J.

    1983-01-01

    The study of spectral line shapes has traditionally been mainly concerned with the measurement and interpretation of absorption or emission profiles. Often only the line widths are studied. The present investigation has the objective to evaluate the additional information which can be obtained by scattering light (usually from a laser) from an atomic system which is being perturbed by collisions. A scattering experiment is discussed. The scattered light consists of two components, a (coherent) Rayleigh component and a redistributed (fluorescent) component. In order to obtain the absorption spectrum, questions regarding the probability of photon absorption are considered. By observing the fluorescence subsequent to absorption during a collision it is found possible to obtain information on the evolution of the system from the point of absorption to the completion of the collision. The information on the intracollisional evolution is the justification for the title of the study, namely 'Why half a collision is better than a whole one'.

  6. Alignment of H(2p) in collisions of protons and antiprotons with hydrogen atoms with screened Coulomb interaction

    NASA Astrophysics Data System (ADS)

    Jakimovski, Dragan; Janev, Ratko K.

    2016-07-01

    The effects of screened Coulomb interaction on the alignment of H(2p) state produced in collisions of hydrogen atoms with protons and antiprotons are investigated in the energy range 1-200 keV by using the two-center atomic orbital close-coupling (TC-AOCC) method. It is shown that the decrease of the binding energy of hydrogen nl-states and the reduction of the number of bound states with increasing the strength of the screening affect significantly the alignment degree and its energy dependence. In the case of antiproton-H collision the difference between the alignments with screened and unscreened Coulomb potential increases with increasing the strength of the screening in the entire energy range above 2 keV/u, while in the case of proton-H collision it does so only in the energy range 5-25 keV/u.

  7. Differential electron-Cu5+ elastic scattering cross sections extracted from electron emission in ion-atom collisions

    NASA Astrophysics Data System (ADS)

    Liao, C.; Hagmann, S.; Bhalla, C. P.; Grabbe, S. R.; Cocke, C. L.; Richard, P.

    1999-04-01

    We present a method of deriving energy and angle-dependent electron-ion elastic scattering cross sections from doubly differential cross sections for electron emission in ion-atom collisions. By analyzing the laboratory frame binary encounter electron production cross sections in energetic ion-atom collisions, we derive projectile frame differential cross sections for electrons elastically scattered from highly charged projectile ions in the range between 60° and 180°. The elastic scattering cross sections are observed to deviate strongly from the Rutherford cross sections for electron scattering from bare nuclei. They exhibit strong Ramsauer-Townsend electron diffraction in the angular distribution of elastically scattered electrons, providing evidence for the strong role of screening played in the collision. Experimental data are compared with partial-wave calculations using the Hartree-Fock model.

  8. Atomic physics experiments at the high energy storage ring

    NASA Astrophysics Data System (ADS)

    Stöhlker, Thomas; Litvinov, Yuri A.; the SPARC Collaboration

    2015-11-01

    Facility for Antiproton and Ion Research (FAIR), will offer unprecedented experimental opportunities. The Stored Particles Atomic Research Collaboration (SPARC) at FAIR aims at creating a worldwide unique research program with highly charged ions by utilizing storage ring and trapping facilities. The foreseen experiments will address physics at strong, ultra-short electromagnetic fields including the fundamental interactions between electrons and heavy nuclei as well as the experiments at the border between nuclear and atomic physics. In view of the staged construction of the FAIR facility, SPARC worked out an early realization scheme for experiments with highly-charged heavy-ions at relativistic energies to be conducted in the High-Energy Storage Ring.

  9. Cold collisions of polyatomic molecular radicals with S-state atoms in a magnetic field: an ab initio study of He + CH2(X) collisions.

    PubMed

    Tscherbul, T V; Grinev, T A; Yu, H-G; Dalgarno, A; Kłos, Jacek; Ma, Lifang; Alexander, Millard H

    2012-09-14

    We develop a rigorous quantum mechanical theory for collisions of polyatomic molecular radicals with S-state atoms in the presence of an external magnetic field. The theory is based on a fully uncoupled space-fixed basis set representation of the multichannel scattering wave function. Explicit expressions are presented for the matrix elements of the scattering Hamiltonian for spin-1/2 and spin-1 polyatomic molecular radicals interacting with structureless targets. The theory is applied to calculate the cross sections and thermal rate constants for spin relaxation in low-temperature collisions of the prototypical organic molecule methylene [CH(2)(X(3)B(1))] with He atoms. To this end, two accurate three-dimensional potential energy surfaces (PESs) of the He-CH(2)(X(3)B(1)) complex are developed using the state-of-the-art coupled-cluster method including single and double excitations along with a perturbative correction for triple excitations and large basis sets. Both PESs exhibit shallow minima and are weakly anisotropic. Our calculations show that spin relaxation in collisions of CH(2), CHD, and CD(2) molecules with He atoms occurs at a much slower rate than elastic scattering over a large range of temperatures (1 μK-1 K) and magnetic fields (0.01-1 T), suggesting excellent prospects for cryogenic helium buffer-gas cooling of ground-state ortho-CH(2)(X(3)B(1)) molecules in a magnetic trap. Furthermore, we find that ortho-CH(2) undergoes collision-induced spin relaxation much more slowly than para-CH(2), which indicates that magnetic trapping can be used to separate nuclear spin isomers of open-shell polyatomic molecules. PMID:22979854

  10. Cold collisions of polyatomic molecular radicals with S-state atoms in a magnetic field: An ab initio study of He + CH2(X~) collisions

    NASA Astrophysics Data System (ADS)

    Tscherbul, T. V.; Grinev, T. A.; Yu, H.-G.; Dalgarno, A.; Kłos, Jacek; Ma, Lifang; Alexander, Millard H.

    2012-09-01

    We develop a rigorous quantum mechanical theory for collisions of polyatomic molecular radicals with S-state atoms in the presence of an external magnetic field. The theory is based on a fully uncoupled space-fixed basis set representation of the multichannel scattering wave function. Explicit expressions are presented for the matrix elements of the scattering Hamiltonian for spin-1/2 and spin-1 polyatomic molecular radicals interacting with structureless targets. The theory is applied to calculate the cross sections and thermal rate constants for spin relaxation in low-temperature collisions of the prototypical organic molecule methylene [CH_2(tilde{X}^3B_1)] with He atoms. To this end, two accurate three-dimensional potential energy surfaces (PESs) of the He-CH_2(tilde{X}^3B_1) complex are developed using the state-of-the-art coupled-cluster method including single and double excitations along with a perturbative correction for triple excitations and large basis sets. Both PESs exhibit shallow minima and are weakly anisotropic. Our calculations show that spin relaxation in collisions of CH2, CHD, and CD2 molecules with He atoms occurs at a much slower rate than elastic scattering over a large range of temperatures (1 μK-1 K) and magnetic fields (0.01-1 T), suggesting excellent prospects for cryogenic helium buffer-gas cooling of ground-state ortho-CH_2(tilde{X}^3B_1) molecules in a magnetic trap. Furthermore, we find that ortho-CH2 undergoes collision-induced spin relaxation much more slowly than para-CH2, which indicates that magnetic trapping can be used to separate nuclear spin isomers of open-shell polyatomic molecules.