Science.gov

Sample records for calculated nuclide compositions

  1. Calculation of the minimum critical mass of fissile nuclides

    SciTech Connect

    Wright, R Q; Hopper, Calvin Mitchell

    2008-01-01

    The OB-1 method for the calculation of the minimum critical mass of fissile actinides in metal/water systems was described in a previous paper. A fit to the calculated minimum critical mass data using the extended criticality parameter is the basis of the revised method. The solution density (grams/liter) for the minimum critical mass is also obtained by a fit to calculated values. Input to the calculation consists of the Maxwellian averaged fission and absorption cross sections and the thermal values of nubar. The revised method gives more accurate values than the original method does for both the minimum critical mass and the solution densities. The OB-1 method has been extended to calculate the uncertainties in the minimum critical mass for 12 different fissile nuclides. The uncertainties for the fission and capture cross sections and the estimated nubar uncertainties are used to determine the uncertainties in the minimum critical mass, either in percent or grams. Results have been obtained for U-233, U-235, Pu-236, Pu-239, Pu-241, Am-242m, Cm-243, Cm-245, Cf-249, Cf-251, Cf-253, and Es-254. Eight of these 12 nuclides are included in the ANS-8.15 standard.

  2. Impact of Nuclear Data Uncertainties on Calculated Spent Fuel Nuclide Inventories and Advanced NDA Instrument Response

    SciTech Connect

    Hu, Jianwei; Gauld, Ian C.

    2014-12-01

    The U.S. Department of Energy’s Next Generation Safeguards Initiative Spent Fuel (NGSI-SF) project is nearing the final phase of developing several advanced nondestructive assay (NDA) instruments designed to measure spent nuclear fuel assemblies for the purpose of improving nuclear safeguards. Current efforts are focusing on calibrating several of these instruments with spent fuel assemblies at two international spent fuel facilities. Modelling and simulation is expected to play an important role in predicting nuclide compositions, neutron and gamma source terms, and instrument responses in order to inform the instrument calibration procedures. As part of NGSI-SF project, this work was carried out to assess the impacts of uncertainties in the nuclear data used in the calculations of spent fuel content, radiation emissions and instrument responses. Nuclear data is an essential part of nuclear fuel burnup and decay codes and nuclear transport codes. Such codes are routinely used for analysis of spent fuel and NDA safeguards instruments. Hence, the uncertainties existing in the nuclear data used in these codes affect the accuracies of such analysis. In addition, nuclear data uncertainties represent the limiting (smallest) uncertainties that can be expected from nuclear code predictions, and therefore define the highest attainable accuracy of the NDA instrument. This work studies the impacts of nuclear data uncertainties on calculated spent fuel nuclide inventories and the associated NDA instrument response. Recently developed methods within the SCALE code system are applied in this study. The Californium Interrogation with Prompt Neutron instrument was selected to illustrate the impact of these uncertainties on NDA instrument response.

  3. Impact of Nuclear Data Uncertainties on Calculated Spent Fuel Nuclide Inventories and Advanced NDA Instrument Response

    DOE PAGESBeta

    Hu, Jianwei; Gauld, Ian C.

    2014-12-01

    The U.S. Department of Energy’s Next Generation Safeguards Initiative Spent Fuel (NGSI-SF) project is nearing the final phase of developing several advanced nondestructive assay (NDA) instruments designed to measure spent nuclear fuel assemblies for the purpose of improving nuclear safeguards. Current efforts are focusing on calibrating several of these instruments with spent fuel assemblies at two international spent fuel facilities. Modelling and simulation is expected to play an important role in predicting nuclide compositions, neutron and gamma source terms, and instrument responses in order to inform the instrument calibration procedures. As part of NGSI-SF project, this work was carried outmore » to assess the impacts of uncertainties in the nuclear data used in the calculations of spent fuel content, radiation emissions and instrument responses. Nuclear data is an essential part of nuclear fuel burnup and decay codes and nuclear transport codes. Such codes are routinely used for analysis of spent fuel and NDA safeguards instruments. Hence, the uncertainties existing in the nuclear data used in these codes affect the accuracies of such analysis. In addition, nuclear data uncertainties represent the limiting (smallest) uncertainties that can be expected from nuclear code predictions, and therefore define the highest attainable accuracy of the NDA instrument. This work studies the impacts of nuclear data uncertainties on calculated spent fuel nuclide inventories and the associated NDA instrument response. Recently developed methods within the SCALE code system are applied in this study. The Californium Interrogation with Prompt Neutron instrument was selected to illustrate the impact of these uncertainties on NDA instrument response.« less

  4. TOF-Bρ mass measurements of very exotic nuclides for astrophysical calculations at the NSCL

    NASA Astrophysics Data System (ADS)

    Matoš, M.; Estrade, A.; Amthor, M.; Aprahamian, A.; Bazin, D.; Becerril, A.; Elliot, T.; Galaviz, D.; Gade, A.; Gupta, S.; Lorusso, G.; Montes, F.; Pereira, J.; Portillo, M.; Rogers, A. M.; Schatz, H.; Shapira, D.; Smith, E.; Stolz, A.; Wallace, M.

    2008-01-01

    Atomic masses play a crucial role in many nuclear astrophysics calculations. The lack of experimental values for relevant exotic nuclides triggered a rapid development of new mass measurement devices around the world. The time-of-flight (TOF) mass measurements offer a complementary technique to the most precise one, Penning trap measurements (Blaum 2006 Phys. Rep. 425 1), the latter being limited by the rate and half-lives of the ions of interest. The NSCL facility provides a well-suited infrastructure for the TOF mass measurements of very exotic nuclei. At this facility, we have recently implemented a TOF-Bρ technique and performed mass measurements of neutron-rich nuclides in the Fe region, important for r-process calculations and for calculations of processes occurring in the crust of accreting neutron stars.

  5. The CAIRN method: automated, reproducible calculation of catchment-averaged denudation rates from cosmogenic nuclide concentrations

    NASA Astrophysics Data System (ADS)

    Marius Mudd, Simon; Harel, Marie-Alice; Hurst, Martin D.; Grieve, Stuart W. D.; Marrero, Shasta M.

    2016-08-01

    We report a new program for calculating catchment-averaged denudation rates from cosmogenic nuclide concentrations. The method (Catchment-Averaged denudatIon Rates from cosmogenic Nuclides: CAIRN) bundles previously reported production scaling and topographic shielding algorithms. In addition, it calculates production and shielding on a pixel-by-pixel basis. We explore the effect of sampling frequency across both azimuth (Δθ) and altitude (Δϕ) angles for topographic shielding and show that in high relief terrain a relatively high sampling frequency is required, with a good balance achieved between accuracy and computational expense at Δθ = 8° and Δϕ = 5°. CAIRN includes both internal and external uncertainty analysis, and is packaged in freely available software in order to facilitate easily reproducible denudation rate estimates. CAIRN calculates denudation rates but also automates catchment averaging of shielding and production, and thus can be used to provide reproducible input parameters for the CRONUS family of online calculators.

  6. Workshop on Cosmogenic Nuclides

    NASA Technical Reports Server (NTRS)

    Reedy, R. C. (Editor); Englert, P. (Editor)

    1986-01-01

    Abstracts of papers presented at the Workshop on Cosmogenic Nuclides are compiled. The major topic areas covered include: new techniques for measuring nuclides such as tandem accelerator and resonance mass spectrometry; solar modulation of cosmic rays; pre-irradiation histories of extraterrestrial materials; terrestrial studies; simulations and cross sections; nuclide production rate calculations; and meteoritic nuclides.

  7. CosmoCalc: An Excel add-in for cosmogenic nuclide calculations

    NASA Astrophysics Data System (ADS)

    Vermeesch, Pieter

    2007-08-01

    As dating methods using Terrestrial Cosmogenic Nuclides (TCN) become more popular, the need arises for a general-purpose and easy-to-use data reduction software. The CosmoCalc Excel add-in calculates TCN production rate scaling factors (using Lal, Stone, Dunai, and Desilets methods); topographic, snow, and self-shielding factors; and exposure ages, erosion rates, and burial ages and visualizes the results on banana-style plots. It uses an internally consistent TCN production equation that is based on the quadruple exponential approach of Granger and Smith (2000). CosmoCalc was designed to be as user-friendly as possible. Although the user interface is extremely simple, the program is also very flexible, and nearly all default parameter values can be changed. To facilitate the comparison of different scaling factors, a set of converter tools is provided, allowing the user to easily convert cut-off rigidities to magnetic inclinations, elevations to atmospheric depths, and so forth. Because it is important to use a consistent set of scaling factors for the sample measurements and the production rate calibration sites, CosmoCalc defines the production rates implicitly, as a function of the original TCN concentrations of the calibration site. The program is best suited for 10Be, 26Al, 3He, and 21Ne calculations, although basic functionality for 36Cl and 14C is also provided. CosmoCalc can be downloaded along with a set of test data from http://cosmocalc.googlepages.com.

  8. Cosmogenic nuclide production rates as a function of latitude and altitude calculated via a physics based model and excitation functions

    NASA Astrophysics Data System (ADS)

    Argento, D.; Reedy, R. C.; Stone, J. O.

    2012-12-01

    Cosmogenic nuclides have been used to develop a set of tools critical to the quantification of a wide range of geomorphic and climatic processes and events (Dunai 2010). Having reliable absolute measurement methods has had great impact on research constraining ice age extents as well as providing important climatic data via well constrained erosion rates, etc. Continuing to improve CN methods is critical for these sciences. While significant progress has been made in the last two decades to reduce uncertainties (Dunai 2010; Gosse & Phillips 2001), numerous aspects still need to be refined in order to achieve the analytic resolution desired by glaciologists and geomorphologists. In order to investigate the finer details of the radiation responsible for cosmogenic nuclide production, we have developed a physics based model which models the radiation cascade of primary and secondary cosmic-rays through the atmosphere. In this study, a Monte Carlo method radiation transport code, MCNPX, is used to model the galactic cosmic-ray (GCR) radiation impinging on the upper atmosphere. Beginning with a spectrum of high energy protons and alpha particles at the top of the atmosphere, the code tracks the primary and resulting secondary particles through a model of the Earth's atmosphere and into the lithosphere. Folding the neutron and proton flux results with energy dependent cross sections for nuclide production provides production rates for key cosmogenic nuclides (Argento et al. 2012, in press; Reedy 2012, in press). Our initial study for high latitude shows that nuclides scale at different rates for each nuclide (Argento 2012, in press). Furthermore, the attenuation length for each of these nuclide production rates increases with altitude, and again, they increase at different rates. This has the consequence of changing the production rate ratio as a function of altitude. The earth's geomagnetic field differentially filters low energy cosmic-rays by deflecting them away

  9. CHARACTERIZATION OF GRAPHITE SLEEVES FROM BUGEY 1 EDF PLANT FOR PERMANENT DISPOSAL--MEASUREMENT AND CALCULATION OF SCALING FACTORS FOR DIFFICULT-TO-MEASURE NUCLIDES

    SciTech Connect

    PONCET, Bernard R.

    2003-02-27

    Electricite De France's Bugey-1 reactor, with graphite moderator, was shutdown permanently in 1994. The natural uranium elements are encased in graphite sleeves to facilitate handling. 2,000 m3 of concrete containers, containing non conditioned graphite sleeves, must be characterized and conditioned before shipment to the national repository site called ''Centre de l'Aube''. The characterization work consists in quantifying Difficult-To-Measure nuclides (DTM) by the use of Scaling Factors (SF), which use Co-60 as tracer. Bugey developed an industrial method for the gamma counting of each package to perform easily and rapidly the measurement of the Co-60 content. Depending upon the DTM radionuclide, Co-60 scaling factors are determined, or by measurement on graphite samples (case of C-14, Cl-36, Ni-63, H-3), either by using a calculation technique which is based upon the impurities present in the graphite sleeves. This method is applied for the other pure beta emitters all DTM radionucli des : Ag-108m, Be-10, Ca-41, Cd-109, Cd-113m, Co-57, Cs-135, Cs-137, Eu-155, Fe-55, Gd-153, Mo-93, Nb- 93m, Nb-94, Ni-59, Pd-107, Pm-147, Sm-151, Sn-119m, Sn-121m, Sn-126, Sr-90, Tc-99, V-49 and Zr-93. Calculations use six sleeve history cases : 1 year at 50% power, 2 years at 50 % power, 3 years at 50 % power, 4 years at 50 % power, 1 year at 100 % power and 2 years at 100 % power. The DTM nuclides have been calculated from impurity concentrations for each of these six cases, and the greatest scaling factor has been kept. The calculation is based upon two impurity sets: First impurity set : a reverse activation calculation provides us with the best estimate value of impurities calculated from the measured mean gamma spectrum and from measured scaling factors. It consists in solving a system of simultaneous equations for the impurities as a function of the mean gamma radioactive spectrum and of the measured scaling factors. The concerned calculated impurities are Co, Cl, Li, Ag, Cs

  10. Absolute isotopic composition of molybdenum and the solar abundances of the p-process nuclides Mo92,94

    NASA Astrophysics Data System (ADS)

    Wieser, M. E.; de Laeter, J. R.

    2007-05-01

    The isotopic composition of molybdenum has been measured with high precision using a thermal ionization mass spectrometer, the linearity of which has been verified by measuring the isotopically-certified reference material for strontium (NIST 987). The abundance sensitivity of the mass spectrometer in the vicinity of the molybdenum ion beams has been carefully examined to ensure the absence of tailing effects. Particular care was given to ensuring that potential isobaric interferences from zirconium and ruthenium did not affect the measurement of the isotopic composition of molybdenum. Gravimetric mixtures of two isotopically enriched isotopes, Mo92 and Mo98, were analyzed mass spectrometrically to calibrate the mass spectrometer, in order to establish the isotope fractionation of the spectrometer for the molybdenum isotopes. This enabled the “absolute” isotopic composition of molybdenum to be determined. An accurate determination of the isotopic composition is required in order to calculate the atomic weight of molybdenum, which is one of the least accurately known values of all the elements. The absolute isotope abundances (in atom %) of molybdenum measured in this experiment are as follows: Mo92=14.5246±0.0015; Mo94=9.1514±0.0074; Mo95=15.8375±0.0098; Mo96=16.672±0.019; Mo97=9.5991±0.0073; Mo98=24.391±0.018; and Mo100=9.824±0.050, with uncertainties at the 1s level. These values enable an atomic weight Ar(Mo) of 95.9602±0.0023 (1s) to be calculated, which is slightly higher than the current Standard Atomic Weight Ar(Mo) =95.94±0.02 and with a much improved uncertainty interval. These “absolute” isotope abundances also enable the Solar System abundances of molybdenum to be calculated for astrophysical purposes. Of particular interest are the Solar System abundances of the two p-process nuclides—Mo92 and Mo94, which are present in far greater abundance than p-process theory suggests. The Solar System abundances for Mo92 and Mo94 of 0.364±0

  11. The procedure and results of calculations of the equilibrium isotopic composition of a demonstration subcritical molten salt reactor

    SciTech Connect

    Nevinitsa, V. A. Dudnikov, A. A.; Blandinskiy, V. Yu.; Balanin, A. L.; Alekseev, P. N.; Titarenko, Yu. E.; Batyaev, V. F.; Pavlov, K. V.; Titarenko, A. Yu.

    2015-12-15

    A subcritical molten salt reactor with an external neutron source is studied computationally as a facility for incineration and transmutation of minor actinides from spent nuclear fuel of reactors of VVER-1000 type and for producing {sup 233}U from {sup 232}Th. The reactor configuration is chosen, the requirements to be imposed on the external neutron source are formulated, and the equilibrium isotopic composition of heavy nuclides and the key parameters of the fuel cycle are calculated.

  12. The procedure and results of calculations of the equilibrium isotopic composition of a demonstration subcritical molten salt reactor

    NASA Astrophysics Data System (ADS)

    Nevinitsa, V. A.; Dudnikov, A. A.; Blandinskiy, V. Yu.; Balanin, A. L.; Alekseev, P. N.; Titarenko, Yu. E.; Batyaev, V. F.; Pavlov, K. V.; Titarenko, A. Yu.

    2015-12-01

    A subcritical molten salt reactor with an external neutron source is studied computationally as a facility for incineration and transmutation of minor actinides from spent nuclear fuel of reactors of VVER-1000 type and for producing 233U from 232Th. The reactor configuration is chosen, the requirements to be imposed on the external neutron source are formulated, and the equilibrium isotopic composition of heavy nuclides and the key parameters of the fuel cycle are calculated.

  13. Factors affecting production rates of cosmogenic nuclides in extraterrestrial matter

    NASA Astrophysics Data System (ADS)

    Reedy, R. C.

    2015-10-01

    Good production rates are needed for cosmic-ray-produced nuclides to interpret their measurements. Rates depend on many factors, especially the pre-atmospheric object's size, the location of the sample in that object (such as near surface or deep inside), and the object's bulk composition. The bulk composition affects rates, especially in objects with very low and very high iron contents. Extraterrestrial materials with high iron contents usually have higher rates for making nuclides made by reactions with energetic particles and lower rates for the capture of thermal neutrons. In small objects and near the surface of objects, the cascade of secondary neutrons is being developed as primary particles are being removed. Deep in large objects, that secondary cascade is fully developed and the fluxes of primary particles are low. Recent work shows that even the shape of an object in space has a small but measureable effect. Work has been done and continues to be done on better understanding those and other factors. More good sets of measurements in meteorites with known exposure geometries in space are needed. With the use of modern Monte Carlo codes for the production and transport of particles, the nature of these effects have been and is being studied. Work needs to be done to improve the results of these calculations, especially the cross sections for making spallogenic nuclides.

  14. a Quantitative Method for Analyzing Radioactive Nuclides in Infinite Composite Materials Using High-Resolution Gamma-Ray Spectroscopy.

    NASA Astrophysics Data System (ADS)

    Day, John Henry, Jr.

    1982-03-01

    A theory is formulated in which the concentration of a radionuclide uniformly distributed throughout an infinite medium is related to the photopeak count rate of a signature gamma ray acquired by a detector within the medium. The mass fraction of the i('th) radionuclide in the medium is given by f(,i) = W(,i)(psi)(,i) (E)/(lamda)(,i)I(,I)(E)K(E); where (psi)(,i)(E) and I(,i)(E) are the observed photopeak count rate and absolute intensity for a gamma-ray emission of energy E. (lamda)(,i) and W(,i) are the decay constant and isotopic mass, respectively. It is shown that the function K(E) is a source volume integration over(' )(epsilon)(E,R)B(E,R)exp( -(SIGMA)(mu)(E)r(R))/(VBAR)R(VBAR)('2) which depends on gamma-ray energy only. Values of the narrow-beam attenuation coefficient (mu) are known for many materials. However, several laboratory experiments are performed in order to obtain data from which to empirically determine the detector response function (epsilon)(E,R)(' )and the gamma-ray build -up-factor(' )B(E,R). Special experimental instrumentation for analyzing radionuclides in infinite composite materials using high -resolution gamma-ray spectrometry is introduced. A probe is constructed which contains a coaxial high-purity germanium crystal to detect the gamma rays, a cryostat to cool the crystal and electronic circuitry to process the signal from the detector. Laboratory models of natural formations are prepared using high-grade radioactive samples diluted with silicon dioxide to obtain the desired concentrations. Each model is sampled to obtain X-ray fluorescence, delayed neutron and fluorimetric analysis from independent laboratories to compare with results using the method presented in this work.

  15. Approximate flash calculations for equation-of-state compositional models

    SciTech Connect

    Nghiem, L.X.; Li, Y.K.

    1985-02-01

    An approximate method for flash calculations (AFC) with an equation of state is presented. The equations for AFC are obtained by linearizing the thermodynamic equilibrium equations at an equilibrium condition termed reference condition. The AFC equations are much simpler than the actual equations for flash calculations and yet give almost the same results. A procedure for generating new reference conditions to keep the AFC results close to the true flash calculation (TFC) results is described. AFC is compared to TFC in the calculation of standard laboratory tests and in the simulation of gas injection processes with a composition model. Excellent results are obtained with AFC in less than half the original execution time.

  16. Nuclide Guide and International Chart of Nuclides - 2008

    NASA Astrophysics Data System (ADS)

    Golashvili, T.

    2009-08-01

    New versions of Nuclide Guide and Chart of the Nuclides were developed as a result of Russian-Chinese collaboration. The Nuclide Guide contains the basic information on more than 3000 radioactive and stable nuclides. The characteristics of isomers with half-lives more than 1 ms are included. For each nuclide spin, parity, mass of nuclide, magnetic moment (if available), mass excess, half-life or abundance, decay modes, branching ratios, emitted particles, energies of most intense gamma-rays and their intensities, decay energies and mean values of radiation energy per decay are given. For stable and natural long-lived nuclides cross-sections of thermal neutron induced activation are indicated. The information presented in the Guide was compiled from 5 sources: 1) ENSDF-2008, 2) atomic mass evaluation-2005 by Audi and Wapstra, 3) interactive data bases at web-sites , , 4) original evaluations of authors, 5) recent publications. The International Chart ot Nuclides was developed on the basis of information presented in Nuclide Guide.

  17. Chart of the Nuclides

    SciTech Connect

    Sartori, Enrico

    1999-03-23

    Nucleus is an interactive PC-based graphical viewer of NUBASE nuclear property data. NUBASE contains experimentally known nuclear properties, together with some values that have been estimated from extrapolation of experimental data for 3010 nuclides. NUBASE also contains data on those isomeric states that have half-lives greater than 1 millisecond; there are 669 such nuclides of which 58 have more than one isomeric state. The latest version of NUCLEUS-CHART has been corrected to include the names and the chemical symbols of the elements 104 to 109 that have been finally adopted by the Commission on Nomenclature of Inorganic Chemistry (CNIC) of the International Union of Pure and Applied Chemistry (IUPAC). They differ from those recommended by the same commission a few years before and that were widely used in the evaluations AME''95 and NUBASE''97. It results in some shuffling of the names and symbols, that may cause confusion in the near future. At AMDC we''ll be as careful as possible to try to avoid such confusion. In advance we apologize if any will occur in the future and recommend the user to always double check these few names.

  18. Chart of the Nuclides

    Energy Science and Technology Software Center (ESTSC)

    1999-03-23

    Nucleus is an interactive PC-based graphical viewer of NUBASE nuclear property data. NUBASE contains experimentally known nuclear properties, together with some values that have been estimated from extrapolation of experimental data for 3010 nuclides. NUBASE also contains data on those isomeric states that have half-lives greater than 1 millisecond; there are 669 such nuclides of which 58 have more than one isomeric state. The latest version of NUCLEUS-CHART has been corrected to include the namesmore » and the chemical symbols of the elements 104 to 109 that have been finally adopted by the Commission on Nomenclature of Inorganic Chemistry (CNIC) of the International Union of Pure and Applied Chemistry (IUPAC). They differ from those recommended by the same commission a few years before and that were widely used in the evaluations AME''95 and NUBASE''97. It results in some shuffling of the names and symbols, that may cause confusion in the near future. At AMDC we''ll be as careful as possible to try to avoid such confusion. In advance we apologize if any will occur in the future and recommend the user to always double check these few names.« less

  19. The computation of body composition data using a programmable calculator.

    PubMed

    Withers, R T

    1986-01-01

    A body composition programme has been developed for the Texas Instruments TI 59 programmable calculator and printer. The methodology involves the determination of body density by underwater weighing with the ventilated residual volume being measured by helium dilution. Some of the labelled output variables included on the printout are: body density, percent body fat, fat mass and fat free mass. PMID:3755094

  20. Cosmogenic nuclide budgeting of floodplain sediment transfer

    NASA Astrophysics Data System (ADS)

    Wittmann, H.; von Blanckenburg, F.

    2009-08-01

    Cosmogenic nuclides produced in quartz may either decay or accumulate while sediment is moved through a river basin. A change in nuclide concentration resulting from storage in a floodplain is potentially important in large drainage basins in which sediment is prone to repeated burial and remobilization as a river migrates through its floodplain. We have modeled depth- and time-dependent cosmogenic nuclide concentration changes for 10Be, 26Al, and 14C during sediment storage and mixing in various active floodplain settings ranging from confined, shallow rivers with small floodplains to foreland-basin scale floodplains traversed by deep rivers. Floodplain storage time, estimated from channel migration rates, ranges from 0.4 kyr for the Beni River basin (Bolivia) to 7 kyr for the Amazon River basin, while floodplain storage depth, estimated from channel depth, ranges from 1 to 25 m. For all modeled active floodplain settings, the long-lived nuclides 10Be and 26Al show neither significant increase in nuclide concentration from irradiation nor decrease from decay. We predict a hypothetical response time after which changes in 10Be or 26Al concentrations become analytically resolvable. This interval ranges from 0.07 to 2 Myr and exceeds in all cases the typical residence time of sediment in a floodplain. Due to the much shorter half life of 14C, nuclide concentrations modeled for the in situ-produced variety of this nuclide are, however, sensitive to floodplain storage on residence times of < 20 kyr. The cosmogenic nuclide composition of old deposits in currently inactive floodplains that have been isolated for periods of millions of years from the river that once deposited them is predicted to either increase or decrease in 10Be and 26Al concentration, depending on the depositional depth. These conditions can be evaluated using the 26Al/ 10Be ratio that readily discloses the depth and duration of storage. We illustrate these models with examples from the Amazon basin

  1. Approximate flash calculations for equation-of-state compositional models--

    SciTech Connect

    Nghiem, L.X.; Li, Y.K. )

    1990-02-01

    An approximate flash-calculation (AFC) method with an equation of state (EOS) is presented. The equations for AFC are obtained by linearizing the thermodynamic equilibrium equations at an equilibrium condition called the reference condition. The AFC equations are much simpler than the actual equations for flash calculations and yet give almost the same results. A procedure for generating new reference conditions to keep the AFC results close to the true flash-calculation (TFC) results is described. AFC is compared with TFC in the calculation of standard laboratory tests and in the simulation of gas-injection processes with a compositional model. Excellent results are obtained with AFC in less than half the original execution time.

  2. Nuclide production by primary cosmic-ray protons

    SciTech Connect

    Reedy, R.C.

    1986-01-01

    The production rates of cosmogenic nuclides in the solar system and in interstellar space were calculated for the primary protons in the galactic and solar cosmic rays. At 1 AU, the long-term average fluxes of solar protons usually produce many more atoms of a cosmogenic nuclide than the primary protons in the galactic cosmic rays (GCR), the exceptions being nuclides made only by high-energy reactions (like /sup 10/Be). Because the particle fluxes inside meteorites and other large objects in space include many secondary neutrons, the production rates are much higher and ratios inside large objects are often very different from those by just the primary GCR protons in small objects. The production rates of cosmogenic nuclides are calculated to vary by about factors of 2.5 during at typical 11-year solar cycle, in agreement with measurements of short-lived radionuclides in recently fallen meteorites. The production of cosmogenic nuclides by the GCR particles outside the heliosphere is higher than that by the modulated GCR primaries normally in the solar system. However, there is considerable uncertainty in the fluxes of interstellar protons and, therefore, in the production rates of cosmogenic nuclides in interstellar space. Production rates and ratios for cosmogenic nuclides would be able to identify particles that were small in space or that were exposed to an unmodulated spectrum of GCR particles. 25 refs., 2 figs., 2 tabs.

  3. Lattice calculation of composite dark matter form factors

    NASA Astrophysics Data System (ADS)

    Appelquist, T.; Brower, R. C.; Buchoff, M. I.; Cheng, M.; Cohen, S. D.; Fleming, G. T.; Kiskis, J.; Lin, M. F.; Neil, E. T.; Osborn, J. C.; Rebbi, C.; Schaich, D.; Schroeder, C.; Syritsyn, S.; Voronov, G.; Vranas, P.; Wasem, J.

    2013-07-01

    Composite dark matter candidates, which can arise from new strongly-coupled sectors, are well-motivated and phenomenologically interesting, particularly in the context of asymmetric generation of the relic density. In this work, we employ lattice calculations to study the electromagnetic form factors of electroweak-neutral dark-matter baryons for a three-color, QCD-like theory with Nf=2 and 6 degenerate fermions in the fundamental representation. We calculate the (connected) charge radius and anomalous magnetic moment, both of which can play a significant role for direct detection of composite dark matter. We find minimal Nf dependence in these quantities. We generate mass-dependent cross sections for dark matter-nucleon interactions and use them in conjunction with experimental results from XENON100, excluding dark matter candidates of this type with masses below 10 TeV.

  4. Application of different nuclides in retrospective dosimetry

    SciTech Connect

    Konheiser, J.; Mittag, S.; Viehrig, H.W.; Gleisberg, B.

    2011-07-01

    The activities of nuclides produced via the neutron irradiation of reactor pressure vessel (RPV) steel are used to validate respective fluence calculations. Niobium, nickel, and technetium isotopes from RPV trepans of the decommissioned NPP Greifswald (VVER-440) have been analyzed. The activities were determined by TRAMO (Monte-Carlo) fluence calculations, newly applying 640 neutron-energy groups and ENDF/B7 data. Relative to earlier results, fluences up to 20% higher have been computed, leading to somewhat better agreement between measurement and calculation, particularly in the case of Tc-99. (authors)

  5. Unconventional Nuclides for Radiopharmaceuticals

    PubMed Central

    Holland, Jason P.; Williamson, Matthew J.; Lewis, Jason S.

    2016-01-01

    Rapid and widespread growth in the use of nuclear medicine for both diagnosis and therapy of disease has been the driving force behind burgeoning research interests in the design of novel radiopharmaceuticals. Until recently, the majority of clinical and basic science research has focused on the development of 11C-, 13N-, 15O-, and 18F-radiopharmaceuticals for use with positron emission tomography (PET) and 99mTc-labeled agents for use with single-photon emission computed tomography (SPECT). With the increased availability of small, low-energy cyclotrons and improvements in both cyclotron targetry and purification chemistries, the use of “nonstandard” radionuclides is becoming more prevalent. This brief review describes the physical characteristics of 60 radionuclides, including β+, β−, γ-ray, and α-particle emitters, which have the potential for use in the design and synthesis of the next generation of diagnostic and/or radiotherapeutic drugs. As the decay processes of many of the radionuclides described herein involve emission of high-energy γ-rays, relevant shielding and radiation safety issues are also considered. In particular, the properties and safety considerations associated with the increasingly prevalent PET nuclides 64Cu, 68Ga, 86Y, 89Zr, and 124I are discussed. PMID:20128994

  6. Composite electron propagator methods for calculating ionization energies.

    PubMed

    Díaz-Tinoco, Manuel; Dolgounitcheva, O; Zakrzewski, V G; Ortiz, J V

    2016-06-14

    Accurate ionization energies of molecules may be determined efficiently with composite electron-propagator (CEP) techniques. These methods estimate the results of a calculation with an advanced correlation method and a large basis set by performing a series of more tractable calculations in which large basis sets are used with simpler approximations and small basis sets are paired with more demanding correlation techniques. The performance of several CEP methods, in which diagonal, second-order electron propagator results with large basis sets are combined with higher-order results obtained with smaller basis sets, has been tested for the ionization energies of closed-shell molecules from the G2 set. Useful compromises of accuracy and computational efficiency employ complete-basis-set extrapolation for second-order results and small basis sets in third-order, partial third-order, renormalized partial-third order, or outer valence Green's function calculations. Analysis of results for vertical as well as adiabatic ionization energies leads to specific recommendations on the best use of regular and composite methods. Results for 22 organic molecules of interest in the design of photovoltaic devices, benzo[a]pyrene, Mg-octaethylporphyrin, and C60 illustrate the capabilities of CEP methods for calculations on large molecules. PMID:27305999

  7. Composite electron propagator methods for calculating ionization energies

    NASA Astrophysics Data System (ADS)

    Díaz-Tinoco, Manuel; Dolgounitcheva, O.; Zakrzewski, V. G.; Ortiz, J. V.

    2016-06-01

    Accurate ionization energies of molecules may be determined efficiently with composite electron-propagator (CEP) techniques. These methods estimate the results of a calculation with an advanced correlation method and a large basis set by performing a series of more tractable calculations in which large basis sets are used with simpler approximations and small basis sets are paired with more demanding correlation techniques. The performance of several CEP methods, in which diagonal, second-order electron propagator results with large basis sets are combined with higher-order results obtained with smaller basis sets, has been tested for the ionization energies of closed-shell molecules from the G2 set. Useful compromises of accuracy and computational efficiency employ complete-basis-set extrapolation for second-order results and small basis sets in third-order, partial third-order, renormalized partial-third order, or outer valence Green's function calculations. Analysis of results for vertical as well as adiabatic ionization energies leads to specific recommendations on the best use of regular and composite methods. Results for 22 organic molecules of interest in the design of photovoltaic devices, benzo[a]pyrene, Mg-octaethylporphyrin, and C60 illustrate the capabilities of CEP methods for calculations on large molecules.

  8. Cosmogenic nuclides: Observable effects of Martian volatiles

    NASA Technical Reports Server (NTRS)

    Reedy, R. C.; Drake, D. M.; Feldman, W. C.

    1988-01-01

    Cosmic-ray produced (cosmogenic) nuclides in returned Martian samples could be used to study the amounts and distributions of volatiles in the recent past on Mars. In planning for the gamma-ray spectrometer experiment that is scheduled to fly on the Mars Observer, many calculations were done on the nuclear reactions that should occur in the Martian surface, studying especially the production and transport of neutrons. It is found that three aspects of Mars can very significantly affect the production of cosmogenic products in Mars: the Martian atmosphere and the presence of H2O in or CO2 on the surface of Mars. These volatile components can greatly affect the energy and spatial distributions of neutrons, expecially those with thermal or near thermal energies, in the surface of Mars. In turn, these neutrons produce many cosmogenic nuclides that can be observed in samples returned from Mars.

  9. Clouds Composition in Super-Earth Atmospheres: Chemical Equilibrium Calculations

    NASA Astrophysics Data System (ADS)

    Kempton, Eliza M.-R.; Mbarek, Rostom

    2015-12-01

    Attempts to determine the composition of super-Earth atmospheres have so far been plagued by the presence of clouds. Yet the theoretical framework to understand these clouds is still in its infancy. For the super-Earth archetype GJ 1214b, KCl, Na2S, and ZnS have been proposed as condensates that would form under the condition of chemical equilibrium, if the planet’s atmosphere has a bulk composition near solar. Condensation chemistry calculations have not been presented for a wider range of atmospheric bulk composition that is to be expected for super-Earth exoplanets. Here we provide a theoretical context for the formation of super-Earth clouds in atmospheres of varied composition by determining which condensates are likely to form, under the assumption of chemical equilibrium. We model super-Earth atmospheres assuming they are formed by degassing of volatiles from a solid planetary core of chondritic material. Given the atomic makeup of these atmospheres, we minimize the global Gibbs free energy of over 550 gases and condensates to obtain the molecular composition of the atmospheres over a temperature range of 350-3,000 K. Clouds should form along the temperature-pressure boundaries where the condensed species appear in our calculations. The super-Earth atmospheres that we study range from highly reducing to oxidizing and have carbon to oxygen (C:O) ratios that are both sub-solar and super-solar, thereby spanning a diverse range of atmospheric composition that is appropriate for low-mass exoplanets. Some condensates appear across all of our models. However, the majority of condensed species appear only over specific ranges of H:O and C:O ratios. We find that for GJ 1214b, KCl is the primary cloud-forming condensate at solar composition, in agreement with previous work. However, for oxidizing atmospheres, where H:O is less than unity, K2SO4 clouds form instead. For carbon-rich atmospheres with super-solar C:O ratios, graphite clouds additionally appear. At

  10. Nuclide Importance and the Steady-State Burnup Equation

    SciTech Connect

    Sekimoto, Hiroshi; Nemoto, Atsushi

    2000-05-15

    Conventional methods for evaluating some characteristic values of nuclides relating to burnup in a given neutron spectrum are reviewed in a mathematically systematic way, and a new method based on the importance theory is proposed. In this method, these characteristic values of a nuclide are equivalent to the importances of the nuclide. By solving the equation adjoint to the steady-state burnup equation with a properly chosen source term, the importances for all nuclides are obtained simultaneously.The fission number importance, net neutron importance, fission neutron importance, and absorbed neutron importance are evaluated and discussed. The net neutron importance is a measure directly estimating neutron economy, and it can be evaluated simply by calculating the fission neutron importance minus the absorbed neutron importance, where only the absorbed neutron importance depends on the fission product. The fission neutron importance and absorbed neutron importance are analyzed separately, and detailed discussions of the fission product effects are given for the absorbed neutron importance.

  11. Solar-Cosmic-Ray-Produced Nuclides in Extraterrestrial Matter

    NASA Technical Reports Server (NTRS)

    Reedy, Robert C.

    2000-01-01

    There are two main types of cosmic rays that have sufficient energy to induce nuclear reactions -- the galactic cosmic rays (GCR) and solar cosmic rays (also called solar energetic particles). Both types of particles can have production rates and production ratios in the small objects often found in cold and hot deserts that are different from those seen for most meteorites, which typically have radii of approx.10-100 centimeters. GCR production rates are often lower than those for most meteorites. GCR production ratios, such as Ne-22/Ne-21, are also often different in small objects. Smaller meteoroids also are more likely to have nuclides made by solar-cosmic-ray (SCR) particles than typically-sized meteorites. The very small meteorite Salem had large amounts of SCR-produced radionuclides. Meteorites recovered in Antarctica are more likely to contain SCR-produced nuclides than other meteorites. Martian and lunar meteorites are also likely to have SCR-produced nuclides. Production rates and profiles for SCR-produced nuclides in meteoroids have been calculated previously. However, the cross sections for the nuclear reactions making many SCR-produced nuclides, such as Be-10, were not well measured then. New rates and profiles are calculated here using good cross sections for the reactions making these nuclides.

  12. Solar-Cosmic-Ray-Produced Nuclides in Extraterrestrial Matter

    NASA Technical Reports Server (NTRS)

    Reedy, Robert C.

    1999-01-01

    There are two main types of cosmic rays that have sufficient energy to induce nuclear reactions -- the galactic cosmic rays (GCR) and solar cosmic rays (also called solar energetic particles). Both types of particles can have production rates and production ratios in the small objects often found in cold and hot deserts that are different from those seen for most meteorites, which typically have radii of approx. 10-100 centimeters. GCR production rates are often lower than those for most meteorites. GCR production ratios, such as Ne-22/Ne-21, are also often different in small objects. Smaller meteoroids also are more likely to have nuclides made by solar-cosmic-ray (SCR) particles than typically-sized meteorites. The very small meteorite Salem had large amounts of SCR-produced radionuclides. Meteorites recovered in Antarctica are more likely to contain SCR-produced nuclides than other meteorites. Martian and lunar meteorites are also likely to have SCR-produced nuclides. Production rates and profiles for SCR-produced nuclides in meteoroids have been calculated previously. However, the cross sections for the nuclear reactions making many SCR-produced nuclides, such as Be-10 were not well measured then. New rates and profiles are calculated here using good cross sections for the reactions making these nuclides.

  13. Calculated stormtime variations in plasmaspheric thermal ion composition

    NASA Technical Reports Server (NTRS)

    Miller, N. J.; Mayr, H. G.; Harris, I.

    1983-01-01

    Model calculations describing stormtime variations in the earth's dayside plasmasphere are used to examine variations in ion composition. The model storm is initiated by high-latitude thermospheric heating that generates meridional winds that carry neutral species, momentum, and energy equatorward. The thermosphere acts on the plasmasphere through collisional transfer of momentum and through chemical reactions between neutral species and ions. Over latitudes near the region of thermospheric heating, the thermosphere-plasmasphere coupling processes cause enhancement in the density of oxygen ions while protons are being lost. Meanwhile, densities of oxygen ions and protons near the equator are increasing together, almost in phase. The largest enhancements in ion density develop at latitudes near 45 deg invariant for both oxygen and hydrogen.

  14. International Chart of the Nuclides - 2003

    SciTech Connect

    Zhao Zhixiang; Zhuang Youxiang; Zhou Chunmei; Huang Xiaolong; Antony, M.S.; Hasegawa, Akira; Katakura, Junichi; Golashvili, T.V.; Kupriyanov, V.M.; Lbov, A.A.; Demidov, A.P.; Chechev, V.P.

    2005-05-24

    The International Chart of Nuclides - 2003 has been developed taking into account the data obtained in 1998 - 2003. Unlike widespread nuclide charts the present Chart of Nuclides contains EVALUATED values of the main characteristics. These values are supplied with the standard deviations. The presented data are applicable in medicine, agriculture, environmental protection etc.

  15. Plumbing Neutron Stars to New Depths with the Binding Energy of the Exotic Nuclide Zn82

    NASA Astrophysics Data System (ADS)

    Wolf, R. N.; Beck, D.; Blaum, K.; Böhm, Ch.; Borgmann, Ch.; Breitenfeldt, M.; Chamel, N.; Goriely, S.; Herfurth, F.; Kowalska, M.; Kreim, S.; Lunney, D.; Manea, V.; Minaya Ramirez, E.; Naimi, S.; Neidherr, D.; Rosenbusch, M.; Schweikhard, L.; Stanja, J.; Wienholtz, F.; Zuber, K.

    2013-01-01

    Modeling the composition of neutron-star crusts depends strongly on binding energies of neutron-rich nuclides near the N=50 and N=82 shell closures. Using a recent development of time-of-flight mass spectrometry for on-line purification of radioactive ion beams to access more exotic species, we have determined for the first time the mass of Zn82 with the ISOLTRAP setup at the ISOLDE-CERN facility. With a robust neutron-star model based on nuclear energy-density-functional theory, we solve the general relativistic Tolman-Oppenheimer-Volkoff equations and calculate the neutron-star crust composition based on the new experimental mass. The composition profile is not only altered but now constrained by experimental data deeper into the crust than before.

  16. A three dimensional calculation of elastic equilibrium for composite materials

    NASA Technical Reports Server (NTRS)

    Lustman, Liviu R.; Rose, Milton E.

    1988-01-01

    A compact scheme is applied to three-dimensional elasticity problems for composite materials, involving simple geometries. The mathematical aspects of this approach are discussed, in particular the iteration method. A vector processor code implementing the compact scheme is presented, and several numerical experiments are summarized.

  17. A three dimensional calculation of elastic equilibrium for composite materials

    NASA Technical Reports Server (NTRS)

    Lustman, Liviu R.; Rose, Milton E.

    1986-01-01

    A compact scheme is applied to three-dimensional elasticity problems for composite materials, involving simple geometries. The mathematical aspects of this approach are discussed, in particular the iteration method. A vector processor code implementing the compact scheme is presented, and several numerical experiments are summarized.

  18. Statistical Uncertainty Analysis Applied to Criticality Calculation

    SciTech Connect

    Hartini, Entin; Andiwijayakusuma, Dinan; Susmikanti, Mike; Nursinta, A. W.

    2010-06-22

    In this paper, we present an uncertainty methodology based on a statistical approach, for assessing uncertainties in criticality prediction using monte carlo method due to uncertainties in the isotopic composition of the fuel. The methodology has been applied to criticality calculations with MCNP5 with additional stochastic input of the isotopic fuel composition. The stochastic input were generated using the latin hypercube sampling method based one the probability density function of each nuclide composition. The automatic passing of the stochastic input to the MCNP and the repeated criticality calculation is made possible by using a python script to link the MCNP and our latin hypercube sampling code.

  19. Simulations of Terrestrial in-situ Cosmogenic-Nuclide Production

    NASA Technical Reports Server (NTRS)

    Reedy, R. C.; Nishiizumi, K.; Lal, D.; Arnold, J. R.; Englert, P. A. J.; Klein, J.; Middleton, R.; Jull, A. J. T.; Donahue, D. J.

    1994-01-01

    Targets of silicon and silicon dioxide were irradiated with spallation neutrons to simulate the production of long-lived radionuclides in the surface of the Earth. Gamma-ray spectroscopy was used to measure Be-7 and Na-22, and accelerator mass spectrometry was used to measure Be-10, C-14, and Al-26. The measured ratios of these nuclides are compared with calculated ratios and with ratios from other simulations and agree well with ratios inferred from terrestrial samples.

  20. Thick-Target Simulation Experiments as a Basis for Consistent Modeling of Cosmogenic Nuclide Production in Extraterrestrial Matter

    NASA Astrophysics Data System (ADS)

    Michel, R.; Lange, H.-J.; Leya, I.; Herpers, U.; Meltzow, B.; Dittrich-Hannen, B.; Suter, M.; Kubik, P. W.

    1995-09-01

    Cosmogenic nuclide production rates in meteoroids depend on size and bulk chemical composition of the meteoroid, on the shielding depth and the chemical composition of a sample in it, on spectral distribution, composition and intensity of solar and galactic cosmic radiation, and on the possibly complex exposure history. Except for bulk and sample chemical compositions, all parameters are unknown and must be reconstructed. In order to interpret cosmogenic nuclide abundances in meteorites with respect to their exposure histories, to reconstruct the preatmospheric shapes of the meteoroids and to draw conclusions about long-term spectral distributions and intensities of the cosmic radiation, reliable model calculations of producton rates must be available. The lack of knowledge about the parameters which influence the production rates causes ambiguity of empirical and physical model calculations, if exclusively meteorite data are taken into account. Physical models of cosmogenic nuclide production in meteoroids without free parameters can be established on the basis of thick-target experiments by which the cosmic ray exposure of meteoroids in space is simulated as close as possible under completely controlled conditions. During recent years, we have performed five such experiments to simulate the exposure of meteoroids to galactic protons [1-6]. Here, we report new results on the latest one of these experiments, in which an artificial iron meteoroid made of steel with a radius of 10 cm was isotropically irradiated by 1.6 GeV protons [4,5]. Measurements and evaluation are now completed for shortand mediumlived radionuclides. Results for long-lived nuclides by AMS and of stable rare gas isotopes are partially available with additional measurements still going on. The results obtained up to now for radionuclide production are presented and discussed with respect to some aspects of the production of cosmogenic nuclides in iron meteoroids and of the influence of bulk

  1. Prediction of fiber composite mechanical behavior made simple. [using a rocket calculator

    NASA Technical Reports Server (NTRS)

    Chamis, C. C.

    1980-01-01

    The elastic properties and failure stresses of angleplied fiber composite laminates were determined using a pocket calculator. The procedure uses simple equations and appropriate graphs of elastic properties versus angle plies, and can handle all types of fiber composites including hybrids. The versatility and generality of the method is illustrated in several step-by-step numerical examples.

  2. Ab initio calculations on magnetism induced by composite defects in magnesium oxide

    SciTech Connect

    Zhang, Yao-Fang; Feng, Min; Shao, Bin; Lu, Yuan; Zuo, Xu; Liu, Hong

    2014-05-07

    The local magnetic state induced by the composite defects, composed of an oxygen vacancy and a nitrogen substituting oxygen, in magnesium oxide has been studied by using ab initio calculation based on density functional theory. The calculated results show that local magnetic moment can be induced by the composite defects around the oxygen vacancy, when the exchange split of the oxygen vacancy is enhanced either by the hybridization between the N-p and nearest neighbor O-p orbitals or by applying on-site Coulomb repulsion (U) and exchange interaction (J). We show that the magnetic state induced by the composite defect is energetically more stable than the non-magnetic state. In addition, we show that the U and J applied on the p-orbitals of N and O atoms may significantly impact the calculated magnetic state of the composite defect, resulting in magnetic state for a configuration that is non-magnetic by generalized gradient approximation.

  3. Cosmogenic Nuclides Study of Large Iron Meteorites

    NASA Astrophysics Data System (ADS)

    Hutzler, A.; Smith, T.; Rochette, P.; Bourles, D. L.; Leya, I.; Gattacceca, J.

    2014-09-01

    Six large iron meteorites were selected (Saint-Aubin, Mont-Dieu, Caille, Morasko, Agoudal, and Gebel Kamil). We measured stable and radiogenic cosmogenic nuclides, to study pre-atmospheric size, cosmic-ray exposure ages and terrestrial ages.

  4. Nuclear fission of neutron-deficient protactinium nuclides

    SciTech Connect

    Nishinaka, I.; Nagame, Y.; Tsukada, K.; Ikezoe, H.; Sueki, K.; Nakahara, H.; Tanikawa, M.; Ohtsuki, T.

    1997-08-01

    Fragment velocity, kinetic energy, mass yield, and element yield distributions in the fission of neutron-deficient Pa isotopes produced in the reactions of {sup 16}O and {sup 18}O on {sup 209}Bi have been measured at incident beam energies near and above the Coulomb barriers by the time-of-flight and radiochemical methods. An asymmetric mass-division component has been observed. Measured fission cross sections were compared with the results of statistical model calculations which take into account two fission barrier heights for symmetric and asymmetric yields. The fission barrier height deduced for the asymmetric fission is found slightly lower than that for the symmetric one. The difference between the two barrier heights in the fission of the present protactinium nuclides (N{approximately}135) is considerably smaller than that in the neutron-rich nuclide of {sup 233}Pa (N{approximately}142), indicating that the difference sensitively depends on the neutron number of the fissioning nuclide. {copyright} {ital 1997} {ital The American Physical Society}

  5. Thermodynamic method of calculating the effect of alloying additives on interphase interaction in composite materials

    NASA Technical Reports Server (NTRS)

    Tuchinsky, L. I.

    1986-01-01

    The effect of alloying additives to the matrix of a composite on the high temperature solubility rate of a single component fiber was analyzed thermodynamically. With an example of binary Ni alloys, with Group IV-VI transition metals reinforced with W fibers, agreement between the calculated and experimental data was demonstrated.

  6. Sensitivity of low energy brachytherapy Monte Carlo dose calculations to uncertainties in human tissue composition

    SciTech Connect

    Landry, Guillaume; Reniers, Brigitte; Murrer, Lars; Lutgens, Ludy; Bloemen-Van Gurp, Esther; Pignol, Jean-Philippe; Keller, Brian; Beaulieu, Luc; Verhaegen, Frank

    2010-10-15

    Purpose: The objective of this work is to assess the sensitivity of Monte Carlo (MC) dose calculations to uncertainties in human tissue composition for a range of low photon energy brachytherapy sources: {sup 125}I, {sup 103}Pd, {sup 131}Cs, and an electronic brachytherapy source (EBS). The low energy photons emitted by these sources make the dosimetry sensitive to variations in tissue atomic number due to the dominance of the photoelectric effect. This work reports dose to a small mass of water in medium D{sub w,m} as opposed to dose to a small mass of medium in medium D{sub m,m}. Methods: Mean adipose, mammary gland, and breast tissues (as uniform mixture of the aforementioned tissues) are investigated as well as compositions corresponding to one standard deviation from the mean. Prostate mean compositions from three different literature sources are also investigated. Three sets of MC simulations are performed with the GEANT4 code: (1) Dose calculations for idealized TG-43-like spherical geometries using point sources. Radial dose profiles obtained in different media are compared to assess the influence of compositional uncertainties. (2) Dose calculations for four clinical prostate LDR brachytherapy permanent seed implants using {sup 125}I seeds (Model 2301, Best Medical, Springfield, VA). The effect of varying the prostate composition in the planning target volume (PTV) is investigated by comparing PTV D{sub 90} values. (3) Dose calculations for four clinical breast LDR brachytherapy permanent seed implants using {sup 103}Pd seeds (Model 2335, Best Medical). The effects of varying the adipose/gland ratio in the PTV and of varying the elemental composition of adipose and gland within one standard deviation of the assumed mean composition are investigated by comparing PTV D{sub 90} values. For (2) and (3), the influence of using the mass density from CT scans instead of unit mass density is also assessed. Results: Results from simulation (1) show that variations

  7. Production systematics of cosmogenic nuclides in the earth

    SciTech Connect

    Reedy, R.C.

    1995-01-01

    The high-energy particles in the galactic cosmic rays, (GCR) can produce nuclides deep in any object exposed to them. These cosmic-ray-produced (cosmogenic) nuclides have been extensively studied during the last four decades, mainly in meteorites and lunar samples (e.g., 1,2). In extraterrestrial matter, several approaches have been used to determine the production systematics of these cosmogenic nuclides. Production rates of most cosmogenic nuclides in the Earth axe much lower, especially those nuclides made ``in situ`` in the Earth`s surface. Many of these @trial cosmogenic nuclides are only now being measured because of improved techniques, such as accelerator mass spectrometry (AMS). There have been very few determinations of the production rates of nuclides made in the Earth by cosmic rays. The work being done for terrestrial cosmogenic nuclides is following the approaches used for, studying the production of extraterrestrial nuclides.

  8. Scan angle calculation and image compositing for the Mexico Forest Mapping Project. Forest Service research note

    SciTech Connect

    Zhu, Z.

    1994-02-01

    Data from the Advanced Very High Resolution Radiometer (AVHRR) were used in a cooperative project, sponsored by the U.S. Department of Agriculture, Forest Service, Southern Forest Experiment Station, and the United Nations, Food and Agriculture Organization (FAO), to map Mexico's forest cover types. To provide satisfactory AVHRR data sets for the project, the sensor scan angle needed to be calculated for data points in the composite image data, and the clouds had to be removed and composite image data created from individual data sets. Techniques used to accomplish those two tasks are described here. Concepts illustrated here should be applicable to other similar projects.

  9. Cosmogenic nuclides in cometary materials: Implications for rate of mass loss and exposure history

    NASA Technical Reports Server (NTRS)

    Herzog, G. F.; Englert, P. A. J.; Reedy, R. C.

    1989-01-01

    As planned, the Rosetta mission will return to earth with a 10-kg core and a 1-kg surface sample from a comet. The selection of a comet with low current activity will maximize the chance of obtaining material altered as little as possible. Current temperature and level of activity, however, may not reliably indicate previous values. Fortunately, from measurements of the cosmogenic nuclide contents of cometary material, one may estimate a rate of mass loss in the past and perhaps learn something about the exposure history of the comet. Perhaps the simplest way to estimate the rate of mass loss is to compare the total inventories of several long-lived cosmogenic radionuclides with the values expected on the basis of model calculations. Although model calculations have become steadily more reliable, application to bodies with the composition of comets will require some extension beyond the normal range of use. In particular, the influence of light elements on the secondary particle cascade will need study, in part through laboratory irradiations of volatile-rich materials. In the analysis of cometary data, it would be valuable to test calculations against measurements of short-lived isotopes.

  10. Benchmark data for validating irradiated fuel compositions used in criticality calculations

    SciTech Connect

    Bierman, S.R.; Talbert, R.J.

    1994-10-01

    To establish criticality safety margins utilizing burnup credit in the storage and transport of spent reactor fuels requires a knowledge of the uncertainty in the calculated fuel composition used in making the reactivity assessment. To provide data for validating such calculated burnup fuel compositions, radiochemical assays have been obtained as part of the United States Department of Energy From-Reactor Cask Development Program. Assay results and associated operating histories on the initial three samples analyzed in this effort are presented. The three samples were taken from different axial regions of a Pressurized Water Reactor fuel rod and represent radiation exposures of about 37, 27, and 44 GWd/MTU. The data are presented in a benchmark type format to facilitate identification/referencing and computer code input.

  11. Accelerator experiments on the contribution of secondary particles to the production of cosmogenic nuclides in meteorites

    NASA Technical Reports Server (NTRS)

    Dragovitsch, P.; Englert, P.

    1985-01-01

    Through the interaction of galactic cosmic particle radiation (GCR) a wide variety of cosmogenic nuclides is produced in meteorites. They provide historical information about the cosmic radiation and the bombarded meteorites. An important way to understand the production mechanisms of cosmogenic nuclides in meteorites is to gather information about the depth and size dependence of the build-up of Galactic Rays Cosmic-secondary particles within meteorites of different sizes and chemical compositions. Simulation experiments with meteorite models offer an alternative to direct observation providing a data basis to describe the development and action of the secondary cascade induced by the GCR in meteorites.

  12. Feasibility on the spectrometric determination of the individual dose rate for detected gamma nuclides using the dose rate spectroscopy

    NASA Astrophysics Data System (ADS)

    Ji, Young-Yong; Chung, Kun Ho; Lee, Wanno; Park, Doo-Won; Kang, Mun-Ja

    2014-04-01

    A spectrometric determination of the dose rate using a detector is a very useful method to identify the contribution of artificial nuclides. In addition, the individual dose rate for detected gamma nuclides from the radioactive materials as well as the environment can give further information such as the in-situ measurement because of the direct relation between the individual dose rate and the activity of a nuclide. In this study, the calculation method for the individual dose rate for detected gamma nuclides was suggested by introducing the concept of the dose rate spectroscopy and the peak-to-total ratio in the energy spectrum for the dose rate, which means just a form of multiplied counts and the value of a G-factor in the spectrum. In addition, the validity of the suggested method for the individual dose rate was experimentally verified through a comparison of the calculation results on the energy spectra for several conditions of the standard source.

  13. A finite element method for shear stresses calculation in composite blade models

    NASA Astrophysics Data System (ADS)

    Paluch, B.

    1991-09-01

    A finite-element method is developed for accurately calculating shear stresses in helicopter blade models, induced by torsion and shearing forces. The method can also be used to compute the equivalent torsional stiffness of the section, their transverse shear coefficient, and the position of their center of torsion. A grid generator method which is a part of the calculation program is also described and used to discretize the sections quickly and to condition the grid data reliably. The finite-element method was validated on a few sections composed of isotropic materials and was then applied to a blade model sections made of composite materials. Good agreement was obtained between the calculated and experimental data.

  14. Structural predictions based on the compositions of cathodic materials by first-principles calculations

    NASA Astrophysics Data System (ADS)

    Li, Yang; Lian, Fang; Chen, Ning; Hao, Zhen-jia; Chou, Kuo-chih

    2015-05-01

    A first-principles method is applied to comparatively study the stability of lithium metal oxides with layered or spinel structures to predict the most energetically favorable structure for different compositions. The binding and reaction energies of the real or virtual layered LiMO2 and spinel LiM2O4 (M = Sc-Cu, Y-Ag, Mg-Sr, and Al-In) are calculated. The effect of element M on the structural stability, especially in the case of multiple-cation compounds, is discussed herein. The calculation results indicate that the phase stability depends on both the binding and reaction energies. The oxidation state of element M also plays a role in determining the dominant structure, i.e., layered or spinel phase. Moreover, calculation-based theoretical predictions of the phase stability of the doped materials agree with the previously reported experimental data.

  15. Corrosion Tests of LWR Fuels - Nuclide Release

    SciTech Connect

    P.A. Finn; Y. Tsai; J.C. Cunnane

    2001-12-14

    Two BWR fuels [64 and 71 (MWd)/kgU], one of which contained 2% Gd, and two PWR fuels [30 and 45 (MWd)/kgU], are tested by dripping groundwater on the fuels under oxidizing and hydrologically unsaturated conditions for times ranging from 2.4 to 8.2 yr at 90 C. The {sup 99}Tc, {sup 129}I, {sup 137}Cs, {sup 97}Mo, and {sup 90}Sr releases are presented to show the effects of long reaction times and of gadolinium on nuclide release. This investigation showed that the five nuclides at long reaction times have similar fractional release rates and that the presence of 2% Gd reduced the {sup 99}Tc cumulative release fraction by about an order of magnitude over that of a fuel with a similar burnup.

  16. Neutron multiplicities for the transplutonium nuclides

    SciTech Connect

    Holden, N.E.; Zucker, M.S.

    1985-01-01

    This paper continues, with respect to the transplutonium nuclides, earlier efforts to collate and evaluate data from the scientific literature on the prompt neutron multiplicity distribution from fission and its first moment = ..sigma..nuPnu. The isotopes considered here for which P/sub nu/ and or data (or both) were found in the literature are of americium (Am), curium (Cm), berkelium (Bk), californium (Cf), einsteinium (Es), fermium (Fm), and nobelium (No).

  17. Calculations of evaporative losses using stable water isotope composition in dry climates

    NASA Astrophysics Data System (ADS)

    Skrzypek, Grzegorz; Mydlowski, Adam; Dogramaci, Shawan; Hedley, Paul; Gibson, John; Grierson, Pauline

    2014-05-01

    Evaporative loss from surface waters is a major component of the hydrological cycle in arid zones, restricting recharge to aquifers and limiting the persistence of surface water bodies. Calculation of evaporative loss is founded on the so-called Craig-Gordon model (C-G), and the stable hydrogen and oxygen isotope composition of water can be successfully used to estimate progressive evaporation. The advantage of this approach is that it does not require monitoring of water levels, inflow and outflow rates. However, the precision and reliability of calculations in very hot and dry climates can be compromised by variable isotope composition of air moisture, which thus needs to be calibrated for C-G model calculations. In this study, we tested the range of uncertainty in the estimation of evaporative losses by cross-validating a simplified stable isotope model with field pan evaporation experiments. The use of standardized pans (1.2 m diameter, max volume 300 dm3) allowed simulation of fast evaporation from shallow water bodies in hot and dry climates (mean daily temperature 29° C and relative humidity between 19 and 26% RH during an 11 day experiment). The stable isotope composition of water in pans changed from -8.23o (δ18O) and -56o (δ2H) to approximately +6.0o (δ18O) and +2.4o (δ2H), reflecting evaporative losses of 56% in sun and 53% in shade. The maximum difference between observed (measured in the field) and calculated evaporative losses was

  18. Characterization of nuclide inventories in waste streams from nuclear power plants

    SciTech Connect

    Oppermann, U.; Mueller, W.

    1993-12-31

    Producers of radioactive waste are increasingly required to characterize the nuclide specific activity inventory of their wastes to demonstrate compliance with the acceptance criteria of interim storages or repositories for the final disposal of radioactive wastes. Nuclide specific characterization of activity inventories for nuclides that are hard to measure in nuclear power plant wastes in general is based on calculations by fixed correlations to easy measurable intense {gamma}-emitters (key nuclides). This method is establish within a CEC project for LWR waste streams from four European countries. First experiences from this project in comparison to data from the US and to earlier evaluations for German LWRs are presented. The applicability of the method is discussed with regard to the measurability of radiologically relevant nuclides comparability between different reactor systems and waste streams, and the availability of the necessary data. All topics are illustrated by examples for individual correlations. Conclusions are drawn for the degree of necessary differentiation and the main factors responsible for these differences.

  19. Significance of the effect of mineral alteration of nuclide migration

    SciTech Connect

    Murakami, Takashi; Ohnuki, Toshihiko; Isobe, Hiroshi; Sato, Tsutomu; Yanase, Nobuyuki; Kimura, Hideo

    1994-12-31

    In order to clarify the effect of mineral alteration on nuclide migration, we examined the processes, mechanisms, and kinetics of chlorite weathering, and the uranium concentrations in minerals and rocks at Koongarra, Australia. The observed concentrations of uranium in rocks were compared to those calculated. The sequence of chlorite weathering may be simply expressed as a chlorite {yields} vermiculite {yields} kaolinite conversion. These minerals occur as a function of depth, which corresponds well to uranium concentrations on the meter scale. Iron minerals, closely related to the uranium redistribution, are released during the weathering. The first-order kinetic model of the weathering process suggests that the weathering rate is not constant but time-dependent. The uranium concentrations are qualitatively proportional to the extent of the weathering, the weathered part having higher uranium concentration. Uranium mainly occurs with iron minerals, and sub micron sized saleeite, a uranyl phosphate, is one of the most probable uranyl phases associated with the iron minerals. The uranium fixation mechanisms are probably saleeite microcrystal coprecipitation and sorption to the iron minerals. Our model, which describes uranium concentrations in rocks as a function of time, shows that the transition zone (a vermiculite dominant area) plays an important role in the uranium migration. We have established that weathering of chlorite has affected the redistribution of uranium for more than one million years. The present study demonstrates the significance of mineral alteration when we estimate nuclide migration for geologic time.

  20. Reliability of the finite element method for calculating free edge stresses in composite laminates

    NASA Technical Reports Server (NTRS)

    Whitcomb, J. D.; Raju, I. S.; Goree, J. G.

    1982-01-01

    The interlaminar normal stress distributions along the interface between the +45 deg and -45 deg plies of a graphite/epoxy laminate, obtained by various investigators, were found to disagree in both magnitude and sign. The reliability of the displacement-formulated finite element method in analyzing the edge-stress problem of a composite laminate is investigated. The history of the edge-stress problem is reviewed, and two well-known elasticity problems, one involving a stress discontinuity and one a singularity, are analyzed. The finite element analysis in these problems yields accurate stress distributions everywhere except in two elements closest to the stress discontinuity or singularity. Stress distributions for a + or -45 deg ply laminate near the singularity were similar to those of the two elasticity problems, demonstrating the methods, accuracy for calculating interlaminar stresses in composite laminates. The disagreement between the numerical methods was attributed to the unsymmetric stress tensor at singularity.

  1. Comment on ''Walker diffusion method for calculation of transport properties of composite materials''

    SciTech Connect

    Kim, In Chan; Cule, Dinko; Torquato, Salvatore

    2000-04-01

    In a recent paper [C. DeW. Van Siclen, Phys. Rev. E 59, 2804 (1999)], a random-walk algorithm was proposed as the best method to calculate transport properties of composite materials. It was claimed that the method is applicable both to discrete and continuum systems. The limitations of the proposed algorithm are analyzed. We show that the algorithm does not capture the peculiarities of continuum systems (e.g., ''necks'' or ''choke points'') and we argue that it is the stochastic analog of the finite-difference method. (c) 2000 The American Physical Society.

  2. Effect of composition on antiphase boundary energy in Ni3Al based alloys: Ab initio calculations

    NASA Astrophysics Data System (ADS)

    Gorbatov, O. I.; Lomaev, I. L.; Gornostyrev, Yu. N.; Ruban, A. V.; Furrer, D.; Venkatesh, V.; Novikov, D. L.; Burlatsky, S. F.

    2016-06-01

    The effect of composition on the antiphase boundary (APB) energy of Ni-based L 12-ordered alloys is investigated by ab initio calculations employing the coherent potential approximation. The calculated APB energies for the {111} and {001} planes reproduce experimental values of the APB energy. The APB energies for the nonstoichiometric γ' phase increase with Al concentration and are in line with the experiment. The magnitude of the alloying effect on the APB energy correlates with the variation of the ordering energy of the alloy according to the alloying element's position in the 3 d row. The elements from the left side of the 3 d row increase the APB energy of the Ni-based L 12-ordered alloys, while the elements from the right side slightly affect it except Ni. The way to predict the effect of an addition on the {111} APB energy in a multicomponent alloy is discussed.

  3. Rock Maker: an MS Excel™ spreadsheet for the calculation of rock compositions from proportional whole rock analyses, mineral compositions, and modal abundance

    NASA Astrophysics Data System (ADS)

    Büttner, Steffen H.

    2012-01-01

    Rock Maker is a simple software tool that computes bulk rock compositions resulting from mixing or unmixing of rocks or minerals. The calculations describe the chemical expression of processes such as magma mixing, fractional crystallization, assimilation, residual melt extraction, or formation of solid solutions. Rock Maker can also be used for the elimination of thermodynamically inactive or unwanted chemical components from the whole rock composition, such as cores of porphyroblasts that are considered not to be in equilibrium with the matrix. The calculation of the resulting rock composition is essentially based on modal proportions and compositions of different components in rocks, which may include specific portions of the rock or individual mineral phases. Compositional data, obtained using XRF, ICPMS, EDS, or EPMA, may include major and trace element concentrations. Depending upon the nature of the problem to be solved, the concentrations of oxidic and elemental components can be added to, or subtracted from, each other, producing the calculated normalized whole rock composition after completion of the investigated process (mixing, unmixing, depletion, enrichment, etc.). Furthermore, the software allows the calculation of whole rock compositions from ideal mineral compositions, for which modal proportions can be chosen from pre-defined mineral compositions. The data set includes the most common rock forming minerals and allows the addition of further phases. This section can be used to calculate the approximate whole rock compositions from petrographic modal analysis. This part of Rock Maker is specifically suitable as a teaching tool that illustrates the interrelationship between mineral compositions, modes, and the corresponding whole rock compositions.

  4. Mass Evaluation for Proton Rich Nuclides

    SciTech Connect

    Wang, M.; Audi, G.; Xu, X.; Pfeiffer, B.; Kondev, F. G.

    2011-11-30

    The Atomic mass evaluation (AME) provides the reliable resource for the values related to atomic masses. Since the publication of the latest version of AME in 2003, many developments for atomic mass determination have been done and important results changed significantly our knowledge. A preliminary version of AME was released in April 2011, and an official version is foreseen to be published in early 2013. The general status of AME is presented and some specific features of AME for proton-rich nuclides are discussed.

  5. Mass measurements of exotic nuclides at SHIPTRAP

    SciTech Connect

    Block, M.; Ackermann, D.; Eliseev, S.; Herfurth, F.; Hessberger, F. P.; Hofmann, S.; Kluge, H.-J.; Maero, G.; Martin, A.; Mazzocco, M.; Mukherjee, M.; Quint, W.; Rahaman, S.; Rauth, C.; Rodriguez, D.; Scheidenberger, C.; Vorobjev, G.; Blaum, K.; Ferrer, R.; Weber, C.

    2007-05-22

    The Penning trap mass spectrometer SHIPTRAP is installed behind the velocity-filter SHIP at GSI for high-precision mass measurements of fusion-evaporation residues. To facilitate an efficient stopping of the reaction products a buffer gas stopping cell is utilized. In an investigation of neutron-deficient nuclides in the terbium-to-thulium region around A {approx_equal} 146, 18 new or improved mass values have been obtained, resulting in a more accurate determination of the proton drip line for holmium and thulium. With the present performance of SHIPTRAP, a first direct mass measurement of transuranium elements in the nobelium region is within reach.

  6. Large-scale erosion rates from in situ-produced cosmogenic nuclides in European river sediments

    NASA Astrophysics Data System (ADS)

    Schaller, M.; von Blanckenburg, F.; Hovius, N.; Kubik, P. W.

    2001-06-01

    We have calculated long-term erosion rates of 20-100 mm/kyr from quartz-contained 10Be in the bedload of middle European rivers for catchments ranging from 10 2 to 10 5 km 2. These rates average over 10-40 kyr and agree broadly with rock uplift, incision and exhumation rates, historic soil erosion rates, and erosion rates calculated from the measured sediment loads of the same rivers. Moreover, our new erosion rate estimates correlate well with lithology and relief. However, in the Regen, Neckar, Loire, and Meuse catchments, cosmogenic nuclide-derived erosion rates are consistently 1.5-4 times greater than the equivalent rates derived from measured river loads. This may be due to the systematic under-representation of high-magnitude, low-frequency transport events in the gauging records which cover less than a century. Alternatively the discrepancy may derive from spatially non-uniform erosion and preferential tapping of deeper sections of the irradiation profile. A third explanation relates the high cosmogenic nuclide-derived erosion rates to inheritance of an elevated Pleistocene erosion signal. Uncertainties associated with the cosmogenic nuclide-derived erosion rate estimates are not greater than the potential errors in conventional estimates. Therefore, the cosmogenic nuclide approach is an effective tool for rapid, catchment-wide assessment of time-integrated rates of bedrock weathering and erosion, and we anticipate its fruitful application to the Quaternary sedimentary record.

  7. Chart of Nuclides from the National Nuclear Data Center (NNDC)

    DOE Data Explorer

    The Chart of Nuclides is a software product that allows users to search and plot nuclear structure and nuclear decay data interactively. The Chart of Nuclides was developed by the National Nuclear Data Center (NNDC). It provides an interface between web users and several databases containing nuclear structure, nuclear decay and some neutron-induced nuclear reaction information. Using the Chart of Nuclides, it is possible to search for nuclear level properties (energy, half-life, spin-parity), gamma-ray information (energy, intensity, multipolarity, coincidences),radiation information following nuclear decay (energy, intensity, dose), and neutron-induced reaction data from the BNL-325 book (thermal cross section and resonance integral). The information provided by the Chart of Nuclides can be seen in tables, level schemes and an interactive chart of nuclides. (From the Chart of Nuclides Description at http://www.nndc.bnl.gov/chart/help/index.jsp?product=chart)

  8. Calculation of compositional dependence of stresses in GaInAs/GaAs strained multilayer heterostructures

    NASA Astrophysics Data System (ADS)

    Nakajima, Kazuo

    1993-02-01

    A theoretical model was proposed to calculate the stress in strained multilayer heterostructures. In this model, each composed crystal layer is divided into many imaginary thin layers. The face force, moment and strained balance were considered over all the imaginary thin layers with coherent interfaces. The accurate bending moment for multilayer heterostructures was derived by expanding Davidenkov's expression of a two-phase composite layer, and it was used in the model. Using this model, the stresses at 25°C were calculated for both the GaInAs/GaAs strained multilayer heterostructure and the GaInAs/GaAs single layer heterostructure, and were compared with each other. In this calculation, the relative thickness of GaInAs layers in the GaInAs/GaAs strained multilayer heterostructure is set up to be equal to that of the GaInAs layer in the GaInAs/GaAs single layer heterostructure. The stress in both the structures was calculated over the entire GaInAs layer composition range. The relative stress in the GaInAs/GaAs bottom heterointerface of the multilayer heterostructure is smaller than that in the GaInAs/GaAs heterointerface of the single layer heterostructure especially for In-rich GaInAs. However, the absolute stress in the GaInAs layer at the bottom heterointerface of the multilayer heterostructure is larger than that in the GaInAs layer at the heterointerface of the single layer heterostructure over the entire GaInAs composition range. The difference between the stresses of both heterostructures increases as the thickness of the GaInAs layer increases. The total thickness of GaInAs layers in the multilayer heterostructure corresponding to a constant interfacial relative stress decreases as the Ga composition in the GaInAs layers decreases and it abruptly decreases when the Ga composition is smaller than 0.4. The relative stress in the GaInAs/GaAs bottom heterointerface of the multilayer heterostructure decreases as the thickness of the GaAs barrier layer

  9. Monte Carlo calculation based on hydrogen composition of the tissue for MV photon radiotherapy.

    PubMed

    Demol, Benjamin; Viard, Romain; Reynaert, Nick

    2015-01-01

    The purpose of this study was to demonstrate that Monte Carlo treatment planning systems require tissue characterization (density and composition) as a function of CT number. A discrete set of tissue classes with a specific composition is introduced. In the current work we demonstrate that, for megavoltage photon radiotherapy, only the hydrogen content of the different tissues is of interest. This conclusion might have an impact on MRI-based dose calculations and on MVCT calibration using tissue substitutes. A stoichiometric calibration was performed, grouping tissues with similar atomic composition into 15 dosimetrically equivalent subsets. To demonstrate the importance of hydrogen, a new scheme was derived, with correct hydrogen content, complemented by oxygen (all elements differing from hydrogen are replaced by oxygen). Mass attenuation coefficients and mass stopping powers for this scheme were calculated and compared to the original scheme. Twenty-five CyberKnife treatment plans were recalculated by an in-house developed Monte Carlo system using tissue density and hydrogen content derived from the CT images. The results were compared to Monte Carlo simulations using the original stoichiometric calibration. Between 300 keV and 3 MeV, the relative difference of mass attenuation coefficients is under 1% within all subsets. Between 10 keV and 20 MeV, the relative difference of mass stopping powers goes up to 5% in hard bone and remains below 2% for all other tissue subsets. Dose-volume histograms (DVHs) of the treatment plans present no visual difference between the two schemes. Relative differences of dose indexes D98, D95, D50, D05, D02, and Dmean were analyzed and a distribution centered around zero and of standard deviation below 2% (3 σ) was established. On the other hand, once the hydrogen content is slightly modified, important dose differences are obtained. Monte Carlo dose planning in the field of megavoltage photon radiotherapy is fully achievable using

  10. Computer program FPIP-REV calculates fission product inventory for U-235 fission

    NASA Technical Reports Server (NTRS)

    Brown, W. S.; Call, D. W.

    1967-01-01

    Computer program calculates fission product inventories and source strengths associated with the operation of U-235 fueled nuclear power reactor. It utilizes a fission-product nuclide library of 254 nuclides, and calculates the time dependent behavior of the fission product nuclides formed by fissioning of U-235.

  11. Assessment of adult body composition using bioelectrical impedance: comparison of researcher calculated to machine outputted values

    PubMed Central

    Franco-Villoria, Maria; Wright, Charlotte M; McColl, John H; Sherriff, Andrea; Pearce, Mark S

    2016-01-01

    Objectives To explore the usefulness of Bioelectrical Impedance Analysis (BIA) for general use by identifying best-evidenced formulae to calculate lean and fat mass, comparing these to historical gold standard data and comparing these results with machine-generated output. In addition, we explored how to best to adjust lean and fat estimates for height and how these overlapped with body mass index (BMI). Design Cross-sectional observational study within population representative cohort study. Setting Urban community, North East England Participants Sample of 506 mothers of children aged 7–8 years, mean age 36.3 years. Methods Participants were measured at a home visit using a portable height measure and leg-to-leg BIA machine (Tanita TBF-300MA). Measures Height, weight, bioelectrical impedance (BIA). Outcome measures Lean and fat mass calculated using best-evidenced published formulae as well as machine-calculated lean and fat mass data. Results Estimates of lean mass were similar to historical results using gold standard methods. When compared with the machine-generated values, there were wide limits of agreement for fat mass and a large relative bias for lean that varied with size. Lean and fat residuals adjusted for height differed little from indices of lean (or fat)/height2. Of 112 women with BMI >30 kg/m2, 100 (91%) also had high fat, but of the 16 with low BMI (<19 kg/m2) only 5 (31%) also had low fat. Conclusions Lean and fat mass calculated from BIA using published formulae produces plausible values and demonstrate good concordance between high BMI and high fat, but these differ substantially from the machine-generated values. Bioelectrical impedance can supply a robust and useful field measure of body composition, so long as the machine-generated output is not used. PMID:26743700

  12. Interpretation of an index of phytoplankton population composition calculated from Remote Airborne Fluorsensor (RAF) data

    NASA Technical Reports Server (NTRS)

    Farmer, F. H.

    1981-01-01

    The calculation of indices of phytoplankton population composition from chlorophyll a fluorescence at 685 nm excited by narrow band light at 454 and 539 nm is discussed. The ratio of the fluorescence excited by light of these two wavelengths is a function of the distribution of the phytoplankton between two color groups, designated the golden-brown and the green. The golden-brown group consists of those species which have the highly photosynthetically active carotenoid-chlorophyll-a-protein complexes, i.e. members of the classes Bacillariophyceae, diatoms Dinophyceae, dinoflagellates, and some members of the class Prymnesiophyceae. The green color group consists those species of phytoplankton which apparently lack those complexes, i.e. members of the classes Chlorophyceae, Euglenophyceae, Prasinophyceae, Eustigmatophyceae, Xanthophyceae, and a few members of the Prymnesiophyceae. A few species of phytoplankton appear to have intermediate characteristics, and would apparently belong to neither group. Most of these species are members of the class Cryptophyceae. The composition index for this class is examined in detail.

  13. A comparison of measured and calculated thermal stresses in a hybrid metal matrix composite spar cap element

    NASA Technical Reports Server (NTRS)

    Jenkins, J. M.; Taylor, A. H.; Sakata, I. F.

    1985-01-01

    A hybrid spar of titanium with an integrally brazed composite, consisting of an aluminum matrix reinforced with boron-carbide-coated fibers, was heated in an oven and the resulting thermal stresses were measured. Uniform heating of the spar in an oven resulted in thermal stresses arising from the effects of dissimilar materials and anisotropy of the metal matrix composite. Thermal stresses were calculated from a finite element structural model using anisotropic material properties deduced from constituent properties and rules of mixtures. Comparisons of calculated thermal stresses with measured thermal stresses on the spar are presented. It was shown that failure to account for anisotropy in the metal matrix composite elements would result in large errors in correlating measured and calculated thermal stresses. It was concluded that very strong material characterization efforts are required to predict accurate thermal stresses in anisotropic composite structures.

  14. Measurements of long-lived cosmogenic nuclides in returned comet nucleus samples

    NASA Technical Reports Server (NTRS)

    Nishiizumi, K.; Kohl, C. P.; Arnold, J. R.

    1989-01-01

    Measurements of long lived cosmic ray produced radionuclides have given much information on the histories and rates of surface evolution for meteorites, the Moon and the Earth. These nuclides can be equally useful in studying cometary histories and post nebular processing of cometary surfaces. The concentration of these nuclides depends on the orbit of the comet (cosmic ray intensity changes with distance from the sun), the depth of the sampling site in the comet surface, and the rate of continuous evolution of the surface (erosion rate of surface materials). If the orbital parameters and the sampling depth are known, production rates of cosmogenic nuclides can be fairly accurately calculated by theoretical models normalized to measurement on lunar surface materials and meteoritic samples. Due to the continuous evaporation of surface materials, it is expected that the long lived radioactivities will be undersaturated. Accurate measurements of the degree of undersaturation in nuclides of different half-lives allows for the determination of the rate of surface material loss over the last few million years.

  15. Cosmogenic nuclides in football-sized rocks.

    NASA Technical Reports Server (NTRS)

    Wahlen, M.; Honda, M.; Imamura, M.; Fruchter, J. S.; Finkel, R. C.; Kohl, C. P.; Arnold, J. R.; Reedy, R. C.

    1972-01-01

    The activity of long- and short-lived isotopes in a series of samples from a vertical column through the center of rock 14321 was measured. Rock 14321 is a 9 kg fragmental rock whose orientation was photographically documented on the lunar surface. Also investigated was a sample from the lower portion of rock 14310, where, in order to study target effects, two different density fractions (mineral separates) were analyzed. A few nuclides in a sample from the comprehensive fines 14259 were measured. This material has been collected largely from the top centimeter of the lunar soil. The study of the deep samples of 14321 and 14310 provided values for the activity of isotopes at points where only effects produced by galactic cosmic rays are significant.

  16. Prompt neutron multiplicities for the transplutonium nuclides

    SciTech Connect

    Holden, N.E.; Zucker, M.S.

    1985-01-01

    The direct determination of the average prompt neutron emission values is reviewed, and a method of comparing different sites of neutron emission multiplicity distribution values is described. Measured and recommended values are tabulated for these nuclides: /sup 241/Am, /sup 242/Am, /sup 242/Cm, /sup 243/Cm, /sup 244/Cm, /sup 246/Cm, /sup 247/Cm, /sup 248/Cm, /sup 250/Cm, /sup 245/Cm, /sup 249/Bk, /sup 246/Cf, /sup 249/Cf, /sup 250/Cf, /sup 252/Cf, /sup 254/Cf, /sup 251/Cf, /sup 253/Es, /sup 254/Es, /sup 244/Fm, /sup 246/Fm, /sup 255/Fm, /sup 252/No, /sup 254/Fm, /sup 256/Fm, /sup 257/Fm. 59 refs., 24 tabs. (LEW)

  17. Nuclide production in (very) small meteorites

    NASA Technical Reports Server (NTRS)

    Arnold, J. R.; Nishiizumi, K.

    1986-01-01

    One of the most interesting open questions in the study of cosmic-ray effects in meteorites is the expected behavior of objects which are very small compared to the mean interaction length of primary galactic cosmic ray (GCR) particles. A reasonable limit might be a pre-atmospheric radius of 5 gram/cm(2), or 1.5 cm for chondrites. These are interesting for at least three reasons: (1) this is a limiting case for large objects, and can help us make better models; (2) this size is intermediate between usual meteorites and irradiated grams (spherules); and (3) these are the most likely objects to show solar cosmic ray (SCR) effects. Reedy (1984) has recently proposed a model for production by GCR of radioactive and stable nuclides in spherical meteorites. Very small objects are expected to deviate from this model in the direction of fewer secondary particles (larger spectral shape parameter), at all depths. The net effect will be significantly lower production of such low-energy products as Mn-53 and Al-26. The SCR production of these and other nuclides will be lower, too, because meteorite orbits extend typically out into the asteroid belt, and the mean SCR flux must fall off approximately as r(-2) with distance from the Sun. Kepler's laws insure that for such orbits most of the exposure time is spent near aphelion. None the less the equivalent mean exposure distance, R(exp), is slightly less than the semimajor axis A because of the weighting by R(-2). For the three meteorite orbits we have, R(exp) has a narrow range, from about 1.6 to 2.1 a.u. This is probably true for the great majority of meteorites.

  18. Cosmogenic nuclides in the Martian surface: Constraints for sample recovery and transport

    NASA Technical Reports Server (NTRS)

    Englert, Peter A. J.

    1988-01-01

    Stable and radioactive cosmogenic nuclides and radiation damage effects such as cosmic ray tracks can provide information on the surface history of Mars. A recent overview on developments in cosmogenic nuclide research for historical studies of predominantly extraterrestrial materials was published previously. The information content of cosmogenic nuclides and radiation damage effects produced in the Martian surface is based on the different ways of interaction of the primary galactic and solar cosmic radiation (GCR, SCR) and the secondary particle cascade. Generally the kind and extent of interactions as seen in the products depend on the following factors: (1) composition, energy and intensity of the primary SCR and GCR; (2) composition, energy and intensity of the GCR-induced cascade of secondary particles; (3) the target geometry, i.e., the spatial parameters of Martian surface features with respect to the primary radiation source; (4) the target chemistry, i.e., the chemical composition of the Martian surface at the sampling location down to the minor element level or lower; and (5) duration of the exposure. These factors are not independent of each other and have a major influence on sample taking strategies and techniques.

  19. Analytical source term optimization for radioactive releases with approximate knowledge of nuclide ratios

    NASA Astrophysics Data System (ADS)

    Hofman, Radek; Seibert, Petra; Kovalets, Ivan; Andronopoulos, Spyros

    2015-04-01

    We are concerned with source term retrieval in the case of an accident in a nuclear power with off-site consequences. The goal is to optimize atmospheric dispersion model inputs using inverse modeling of gamma dose rate measurements (instantaneous or time-integrated). These are the most abundant type of measurements provided by various radiation monitoring networks across Europe and available continuously in near-real time. Usually, a source term of an accidental release comprises of a mixture of nuclides. Unfortunately, gamma dose rate measurements do not provide a direct information on the source term composition; however, physical properties of respective nuclides (deposition properties, decay half-life) can yield some insight. In the method presented, we assume that nuclide ratios are known at least approximately, e.g. from nuclide specific observations or reactor inventory and assumptions on the accident type. The source term can be in multiple phases, each being characterized by constant nuclide ratios. The method is an extension of a well-established source term inversion approach based on the optimization of an objective function (minimization of a cost function). This function has two quadratic terms: mismatch between model and measurements weighted by an observation error covariance matrix and the deviation of the solution from a first guess weighted by the first-guess error covariance matrix. For simplicity, both error covariance matrices are approximated as diagonal. Analytical minimization of the cost function leads to a liner system of equations. Possible negative parts of the solution are iteratively removed by the means of first guess error variance reduction. Nuclide ratios enter the problem in the form of additional linear equations, where the deviations from prescribed ratios are weighted by factors; the corresponding error variance allows us to control how strongly we want to impose the prescribed ratios. This introduces some freedom into the

  20. Effect of elemental compositions on Monte Carlo dose calculations in proton therapy of eye tumors

    NASA Astrophysics Data System (ADS)

    Rasouli, Fatemeh S.; Farhad Masoudi, S.; Keshazare, Shiva; Jette, David

    2015-12-01

    Recent studies in eye plaque brachytherapy have found considerable differences between the dosimetric results by using a water phantom, and a complete human eye model. Since the eye continues to be simulated as water-equivalent tissue in the proton therapy literature, a similar study for investigating such a difference in treating eye tumors by protons is indispensable. The present study inquires into this effect in proton therapy utilizing Monte Carlo simulations. A three-dimensional eye model with elemental compositions is simulated and used to examine the dose deposition to the phantom. The beam is planned to pass through a designed beam line to moderate the protons to the desired energies for ocular treatments. The results are compared with similar irradiation to a water phantom, as well as to a material with uniform density throughout the whole volume. Spread-out Bragg peaks (SOBPs) are created by adding pristine peaks to cover a typical tumor volume. Moreover, the corresponding beam parameters recommended by the ICRU are calculated, and the isodose curves are computed. The results show that the maximum dose deposited in ocular media is approximately 5-7% more than in the water phantom, and about 1-1.5% less than in the homogenized material of density 1.05 g cm-3. Furthermore, there is about a 0.2 mm shift in the Bragg peak due to the tissue composition difference between the models. It is found that using the weighted dose profiles optimized in a water phantom for the realistic eye model leads to a small disturbance of the SOBP plateau dose. In spite of the plaque brachytherapy results for treatment of eye tumors, it is found that the differences between the simplified models presented in this work, especially the phantom containing the homogenized material, are not clinically significant in proton therapy. Taking into account the intrinsic uncertainty of the patient dose calculation for protons, and practical problems corresponding to applying patient

  1. Constraints in calculations of evaporative losses in arid climates using the stable isotope composition of water

    NASA Astrophysics Data System (ADS)

    Skrzypek, G.; Mydlowski, A.; Dogramaci, S.; Hedley, P.; Gibson, J. J.; Grierson, P. F.

    2014-12-01

    Accurate quantification of evaporative losses to the atmosphere from surface water bodies is essential for calibration and validation of hydrological models, particularly in remote arid and semi-arid regions, where rivers and lakes are generally minimally gauged. In this study, we reviewed and combined the most recent equations for estimation of evaporative losses based on the revised Craig-Gordon model. We designed new software, called Hydrocalculator, which allows quick and robust estimation of evaporative losses based on the isotopic composition of water. We validated Hydrocalculator by testing the range of uncertainty in the estimation of evaporative losses in arid climates by cross-validating a simplified stable isotope model with field pan evaporation experiments. The use of standardized pans (1.2 m diameter, volume 300 dm3) in hot and dry climates (temperature 29°C and relative humidity between 19 and 26%) allowed simulation of fast evaporation from shallow water bodies. Several factors may contribute to the uncertainty in the evaporative loss calculations. The analytical uncertainty in the determination of the stable isotope composition of water may contribute to ~0.6% for δ18O and ~1.4% for δ2H. The model is less sensitive to uncertainty in climatic variables and an uncertainty of 1°C in air temperature will result only in the ~0.1% uncertainty in δ18O and δ2H. However, uncertainty in relative humidity of 10% will result in an uncertainty in the final outcome of 0.4% (δ18O) and 1.0% (δ2H). Significantly higher uncertainty in evaporative loss estimation is thus associated with uncertainty in ambient air moisture estimation or analysis. An error of 20‰ in δ2H and 5.0‰ in δ18O will result in a maximum difference of 2.4% (δ2H) and 1.7% (δ18O) in the final calculations. Hydrocalculator can thus provide accurate, rapid and cost-effective insight into the water balance of surface water pools. We used the new software to determine the origin of

  2. Nuclide analysis in high burnup fuel samples irradiated in Vandellós 2

    NASA Astrophysics Data System (ADS)

    Zwicky, H. U.; Low, J.; Granfors, M.; Alejano, C.; Conde, J. M.; Casado, C.; Sabater, J.; Lloret, M.; Quecedo, M.; Gago, J. A.

    2010-07-01

    In the framework of a high burnup fuel demonstration programme, rods with an enrichment of 4.5% 235U were operated to a rod average burnup of about 70 MWd/kgU in the Spanish Vandellós 2 pressurised water reactor. The rods were sent to hot cells and used for different research projects. This paper describes the isotopic composition measurements performed on samples of those rods, and the analysis of the measurement results based on comparison against calculated values. The fraction and composition of fission gases released to the rod free volume was determined for two of the rods. About 8% of Kr and Xe produced by fission were released. From the isotopic composition of the gases, it could be concluded that the gases were not preferentially released from the peripheral part of the fuel column. Local burnup and isotopic content of gamma emitting nuclides were determined by quantitatively evaluating axial gamma scans of the full rods. Nine samples were cut at different axial levels from three of the rods and analysed in two campaigns. More than 50 isotopes of 16 different elements were assessed, most of them by Inductively Coupled Plasma Mass Spectrometry after separation with High Performance Liquid Chromatography. In general, these over 400 data points gave a consistent picture of the isotopic content of irradiated fuel as a function of burnup. Only in a few cases, the analysis provided unexpected results that seem to be wrong, in most cases due to unidentified reasons. Sample burnup analysis was performed by comparing experimental isotopic abundances of uranium and plutonium composition as well as neodymium isotopic concentrations with corresponding CASMO based data. The results were in agreement with values derived independently from gamma scanning and from core design data and plant operating records. Measured isotope abundances were finally assessed using the industry standard SAS2H sequence of the SCALE code system. This exercise showed good agreement between

  3. Sensitivity Analysis of Nuclide Importance to One-Group Neutron Cross Sections

    SciTech Connect

    Sekimoto, Hiroshi; Nemoto, Atsushi; Yoshimura, Yoshikane

    2001-07-15

    The importance of nuclides is useful when investigating nuclide characteristics in a given neutron spectrum. However, it is derived using one-group microscopic cross sections, which may contain large errors or uncertainties. The sensitivity coefficient shows the effect of these errors or uncertainties on the importance.The equations for calculating sensitivity coefficients of importance to one-group nuclear constants are derived using the perturbation method. Numerical values are also evaluated for some important cases for fast and thermal reactor systems.Many characteristics of the sensitivity coefficients are derived from the derived equations and numerical results. The matrix of sensitivity coefficients seems diagonally dominant. However, it is not always satisfied in a detailed structure. The detailed structure of the matrix and the characteristics of coefficients are given.By using the obtained sensitivity coefficients, some demonstration calculations have been performed. The effects of error and uncertainty of nuclear data and of the change of one-group cross-section input caused by fuel design changes through the neutron spectrum are investigated. These calculations show that the sensitivity coefficient is useful when evaluating error or uncertainty of nuclide importance caused by the cross-section data error or uncertainty and when checking effectiveness of fuel cell or core design change for improving neutron economy.

  4. Approach for validating actinide and fission product compositions for burnup credit criticality safety analyses

    SciTech Connect

    Radulescu, Georgeta; Gauld, Ian C.; Ilas, Germina; Wagner, John C.

    2014-11-01

    This paper describes a depletion code validation approach for criticality safety analysis using burnup credit for actinide and fission product nuclides in spent nuclear fuel (SNF) compositions. The technical basis for determining the uncertainties in the calculated nuclide concentrations is comparison of calculations to available measurements obtained from destructive radiochemical assay of SNF samples. Probability distributions developed for the uncertainties in the calculated nuclide concentrations were applied to the SNF compositions of a criticality safety analysis model by the use of a Monte Carlo uncertainty sampling method to determine bias and bias uncertainty in effective neutron multiplication factor. Application of the Monte Carlo uncertainty sampling approach is demonstrated for representative criticality safety analysis models of pressurized water reactor spent fuel pool storage racks and transportation packages using burnup-dependent nuclide concentrations calculated with SCALE 6.1 and the ENDF/B-VII nuclear data. Furthermore, the validation approach and results support a recent revision of the U.S. Nuclear Regulatory Commission Interim Staff Guidance 8.

  5. Approach for validating actinide and fission product compositions for burnup credit criticality safety analyses

    DOE PAGESBeta

    Radulescu, Georgeta; Gauld, Ian C.; Ilas, Germina; Wagner, John C.

    2014-11-01

    This paper describes a depletion code validation approach for criticality safety analysis using burnup credit for actinide and fission product nuclides in spent nuclear fuel (SNF) compositions. The technical basis for determining the uncertainties in the calculated nuclide concentrations is comparison of calculations to available measurements obtained from destructive radiochemical assay of SNF samples. Probability distributions developed for the uncertainties in the calculated nuclide concentrations were applied to the SNF compositions of a criticality safety analysis model by the use of a Monte Carlo uncertainty sampling method to determine bias and bias uncertainty in effective neutron multiplication factor. Application ofmore » the Monte Carlo uncertainty sampling approach is demonstrated for representative criticality safety analysis models of pressurized water reactor spent fuel pool storage racks and transportation packages using burnup-dependent nuclide concentrations calculated with SCALE 6.1 and the ENDF/B-VII nuclear data. Furthermore, the validation approach and results support a recent revision of the U.S. Nuclear Regulatory Commission Interim Staff Guidance 8.« less

  6. Modeling for calculation of vanadium oxide film composition in reactive-sputtering process

    SciTech Connect

    Yu He; Jiang Yadong; Wang Tao; Wu Zhiming; Yu Junsheng; Wei Xiongbang

    2010-05-15

    A modified model describing the changing ratio of vanadium to oxide on the target and substrate as a function of oxygen flow is described. Actually, this ratio is extremely sensitive to the deposition conditions during the vanadium oxide (VO{sub x}) reactive magnetron-sputtering process. The method in this article is an extension of a previously presented Berg's model, where only a single stoichiometry compound layer was taken into consideration. This work deals with reactive magnetron sputtering of vanadium oxide films with different oxygen contents from vanadium metal target. The presence of vanadium mixed oxides at both target and substrate surface produced during reactive-sputtering process are included. It shows that the model can be used for the optimization of film composition with respect to oxygen flow in a stable hysteresis-free reactive-sputtering process. A systematic experimental study of deposition rate of VO{sub x} with respect to target ion current was also made. Compared to experimental results, it was verified that the theoretical calculation from modeling is in good agreement with the experimental counterpart.

  7. Reportable Nuclide Criteria for ORNL Radioactive Waste Management Activities - 13005

    SciTech Connect

    McDowell, Kip; Forrester, Tim; Saunders, Mark

    2013-07-01

    The U.S. Department of Energy's Oak Ridge National Laboratory (ORNL) in Oak Ridge, Tennessee generates numerous radioactive waste streams. Many of those streams contain a large number of radionuclides with an extremely broad range of concentrations. To feasibly manage the radionuclide information, ORNL developed reportable nuclide criteria to distinguish between those nuclides in a waste stream that require waste tracking versus those nuclides of such minimal activity that do not require tracking. The criteria include tracking thresholds drawn from ORNL onsite management requirements, transportation requirements, and relevant treatment and disposal facility acceptance criteria. As a management practice, ORNL maintains waste tracking on a nuclide in a specific waste stream if it exceeds any of the reportable nuclide criteria. Nuclides in a specific waste stream that screen out as non-reportable under all these criteria may be dropped from ORNL waste tracking. The benefit of these criteria is to ensure that nuclides in a waste stream with activities which meaningfully affect safety and compliance are tracked, while documenting the basis for removing certain isotopes from further consideration. (authors)

  8. Reportable Nuclide Criteria for ORNL Waste Management Activities - 13005

    SciTech Connect

    McDowell, Kip; Forrester, Tim; Saunders, Mark Edward

    2013-01-01

    The U.S. Department of Energy's Oak Ridge National Laboratory (ORNL) in Oak Ridge, Tennessee generates numerous radioactive waste streams. Many of those streams contain a large number of radionuclides with an extremely broad range of concentrations. To feasibly manage the radionuclide information, ORNL developed a reportable nuclide criteria to distinguish between those nuclides in a waste stream that require waste tracking versus those nuclides of such minimal activity that do not require tracking. The criteria include tracking thresholds drawn from ORNL onsite management requirements, transportation requirements, and relevant treatment and disposal facility acceptance criteria. As a management practice, ORNL maintains waste tracking on a nuclide in a specific waste stream if it exceeds any of the reportable nuclide criteria. Nuclides in a specific waste stream that screen out as non-reportable under all these criteria may be dropped from ORNL waste tracking. The benefit of this criteria is to ensure that nuclides in a waste stream with activities which meaningfully affect safety and compliance are tracked, while documenting the basis for removing certain isotopes from further consideration.

  9. Alpha-emitting nuclides in the marine environment

    NASA Astrophysics Data System (ADS)

    Pentreath, R. J.

    1984-06-01

    The occurrence of alpha-emitting nuclides and their daughter products in the marine environment continues to be a subject of study for many reasons. Those nuclides which occur naturally, in the uranium, thorium and actinium series, are of interest because of their value in determining the rates of geological and geochemical processes in the oceans. Studies of them address such problems as the determination of rates of transfer of particulate matter, deposition rates, bioturbation rates, and so on. Two of the natural alpha-series nuclides in which a different interest has been expressed are 210Po and 226Ra, because their concentrations in marine organisms are such that they contribute to a significant fraction of the background dose rates sustained both by the organisms themselves and by consumers of marine fish and shellfish. To this pool of naturally-occurring nuclides, human activities have added the transuranium nuclides, both from the atmospheric testing of nuclear devices and from the authorized discharges of radioactive wastes into coastal waters and the deep sea. Studies have therefore been made to understand the chemistry of these radionuclides in sea water, their association with sedimentary materials, and their accumulation by marine organisms, the last of these being of particular interest because the transuranics are essentially "novel" elements to the marine fauna and flora. The need to predict the long-term behaviour of these nuclides has, in turn, stimulated research on those naturally-occurring nuclides which may behave in a similar manner.

  10. Depth and size effects on cosmogenic nuclide production in meteorites

    NASA Technical Reports Server (NTRS)

    Englert, P.

    1985-01-01

    The galactic cosmic particle radiation (GCR) can cause changes in condensed extraterrestrial matter in different ways. It can lose energy via ionization processes of induced nuclear reactions which lead to a wide variety of stable and radioactive cosmogenic nuclides. Heavy particles incur radiation damage in minerals such as olivine and pyroxene. Light particles predominantly tend to induce nuclear reactions, causing the development of a secondary particle cascade of neutrons, protons, pions and gamma-rays and the production of cosmogenic nuclides. Such processes are described by various models, which predict the depth and size dependent production of cosmogenic nuclides.

  11. NEANSC international evaluation cooperation SG10 activities on inelastic scattering cross sections for weakly absorbing fission-product nuclides

    SciTech Connect

    Kawai, Masayoshi; Chiba, Satoshi; Nakagawa, Tsuneo; Nakajima, Yutaka; Zukeran, Atsushi; Gruppelaar, H.; Hogenbirk, A.; Salvatores, M.; Dietze, K.

    1994-12-31

    An evaluation method of inelastic scattering cross sections of FP nuclides is investigated. The origins of the discrepancy found in the calculated and measured sample reactivity worths are also discussed emphasizing the effect of ambiguity in inelastic scattering cross sections and neutron spectra.

  12. Light mass elements total half-lives for selected long-lived nuclides

    NASA Astrophysics Data System (ADS)

    Holden, N. E.

    In the past, many compilations and evaluations of half lives have been made which have uncritically accepted authors' values and uncertainties. They have merely recommended weight averaged reported results. This evaluation attempts to reanalyze each experiment in the literature including an estimate of the standard deviation utilizing, where possible, an estimate of the systematic error. This paper constitutes a preliminary step in the process of recommending values. The long lived nuclides of light elements are of interest for their use in dating methods and for calculating cosmic ray exposure ages of meteorites. Experimental data on the half lives of selected nuclides have been evaluated and recommended values and uncertainties are presented for the following nuclides: (3)H, (10)Be, (14)C, (26)Al, (39)Ar, (40)K, (50)V, (53)Mn, (76)Ge, (87)Eb, (92)Nb, (107)Pd, (113)Cd, (115)In and (123)Te. The impact of the recommended (14)C half life of 5715 years on the carbon dating techniques, which uses the Libby value of 5568 years, will be discussed. Also the possible primordial occurrence of (92)Nb is now definitely ruled out by the recommended half life of 3.7 x 10(7). Finally, based on the recommended (26)Al half life value, the (21)Ne production rate for calculating cosmic ray exposure ages remains too high, compared to rates using the (53)Mn and (10)Be half life values.

  13. The even-odd systematics in R-process nuclide abundances

    NASA Technical Reports Server (NTRS)

    Marti, K.; Suess, H. E.

    1988-01-01

    The paper reports and discusses solar system N(R) abundances for nuclides A greater than 70, obtained as differences between measured solar system abundances and calculated S-process contributions. The abundance peak at A of about 163 in the rare earth element region reveals properties which are similar to those of the R-process peaks corresponding to magic neutron numbers N = 82 and N = 126. Systematic differences in the N(R) abundances of even-A and odd-A nuclides are restricted to specific mass regions. It is concluded that these differences are most probably related to the properties of nuclear species during beta(-) decay to the stability valley.

  14. Calculation of the relative uniformity coefficient on the green composites reinforced with cotton and hemp fabric

    NASA Astrophysics Data System (ADS)

    Baciu, Florin; Hadǎr, Anton; Sava, Mihaela; Marinel, Stǎnescu Marius; Bolcu, Dumitru

    2016-06-01

    In this paper it is studied the influence of discontinuities on elastic and mechanical properties of green composite materials (reinforced with fabric of cotton or hemp). In addition, it is studied the way variations of the volume f the reinforcement influences the elasticity modulus and the tensile strength for the studied composite materials. In order to appreciate the difference in properties between different areas of the composite material, and also the dimensions of the defective areas, we have introduced a relative uniformity coefficient with which the mechanical behavior of the studied composite is compared with a reference composite. To validate the theoretical results we have obtained we made some experiments, using green composites reinforced with fabric, with different imperfection introduced special by cutting the fabric.

  15. PRODUCTION CONSIDERATIONS FOR THE CLASSICAL PET NUCLIDES.

    SciTech Connect

    FINN,R.; SCHLYER,D.

    2001-06-25

    Nuclear Medicine is the specialty of medical imaging, which utilizes a variety of radionuclides incorporated into specific compounds for diagnostic imaging and therapeutic applications. During recent years, research efforts associated with this discipline have concentrated on the decay characteristics of particular radionuclides and the design of unique radiolabeled tracers necessary to achieve time-dependent molecular images. The specialty is expanding with specific Positron emission tomography (PET) and SPECT radiopharmaceuticals allowing for an extension from functional process imaging in tissue to pathologic processes and nuclide directed treatments. PET is an example of a technique that has been shown to yield the physiologic information necessary for clinical oncology diagnoses based upon altered tissue metabolism. Most PET drugs are currently produced using a cyclotron at locations that are in close proximity to the hospital or academic center at which the radiopharmaceutical will be administered. In November 1997, a law was enacted called the Food and Drug Administration Modernization Act of 1997 which directed the Food and Drug Administration (FDA) to establish appropriate procedures for the approval of PET drugs in accordance with section 505 of the Federal Food, Drug, and Cosmetic Act and to establish current good manufacturing practice requirements for such drugs. At this time the FDA is considering adopting special approval procedures and cGMP requirements for PET drugs. The evolution of PET radiopharmaceuticals has introduced a new class of ''drugs'' requiring production facilities and product formulations that must be closely aligned with the scheduled clinical utilization. The production of the radionuclide in the appropriate synthetic form is but one critical component in the manufacture of the finished radiopharmaceutical.

  16. Production and Recoil Loss of Cosmogenic Nuclides in Presolar Grains

    NASA Astrophysics Data System (ADS)

    Trappitsch, Reto; Leya, Ingo

    2016-05-01

    Presolar grains are small particles that condensed in the vicinity of dying stars. Some of these grains survived the voyage through the interstellar medium (ISM) and were incorporated into meteorite parent bodies at the formation of the Solar System. An important question is when these stellar processes happened, i.e., how long presolar grains were drifting through the ISM. While conventional radiometric dating of such small grains is very difficult, presolar grains are irradiated with galactic cosmic rays (GCRs) in the ISM, which induce the production of cosmogenic nuclides. This opens the possibility to determine cosmic-ray exposure (CRE) ages, i.e., how long presolar grains were irradiated in the ISM. Here, we present a new model for the production and loss of cosmogenic 3He, 6,7Li, and 21,22Ne in presolar SiC grains. The cosmogenic production rates are calculated using a state-of-the-art nuclear cross-section database and a GCR spectrum in the ISM consistent with recent Voyager data. Our findings are that previously measured 3He and 21Ne CRE ages agree within the (sometimes large) 2σ uncertainties and that the CRE ages for most presolar grains are smaller than the predicted survival times. The obtained results are relatively robust since interferences from implanted low-energy GCRs into the presolar SiC grains and/or from cosmogenic production within the meteoroid can be neglected.

  17. (The fate of nuclides in natural water systems)

    SciTech Connect

    Turekian, K.K. . Dept. of Geology and Geophysics)

    1989-01-01

    Our research at Yale on the fate of nuclides in natural water systems has three components to it: the study of the atmospheric precipitation of radionuclides and other chemical species; the study of the behavior of natural radionuclides in groundwater and hydrothermal systems; and understanding the controls on the distribution of radionuclides and stable nuclides in the marine realm. In this section a review of our progress in each of these areas is presented.

  18. Thermodynamic calculation and interatomic potential to predict the favored composition region for the Cu-Zr-Al metallic glass formation.

    PubMed

    Cui, Y Y; Wang, T L; Li, J H; Dai, Y; Liu, B X

    2011-03-01

    For the Cu-Zr-Al system, the glass forming compositions were firstly calculated based on the extended Miedema's model, suggesting that the amorphous phase could be thermodynamically favored over a large composition region. An n-body potential was then constructed under the smoothed and long-range second-moment-approximation of tight-binding formulism. Applying the constructed Cu-Zr-Al potential, molecular dynamics simulations were conducted using solid solution models to compare relative stability of crystalline solid solution versus its disordered counterpart. Simulations reveal that the physical origin of metallic glass formation is crystalline lattice collapsing while solute concentration exceeding the critical value, thus predicting a hexagonal composition region, within which the Cu-Zr-Al ternary metallic glass formation is energetically favored. The molecular dynamics simulations predicted composition region is defined as the quantitative glass-forming-ability or glass-forming-region of the Cu-Zr-Al system. PMID:21229150

  19. Nuclear Properties and Decay Data Chart of Nuclides.

    Energy Science and Technology Software Center (ESTSC)

    2008-04-04

    Version 00 NUCHART displays nuclear decay data graphically on a PC and, includes a search routine for assigning gamma-ray energies to radionuclides. The numerical data included in NUCHART were taken from the online database "NUDAT" Version of March 1994. The following information is presented: (1) Nuclide information: for each nuclide, abundance, mass excess, (main) decay mode, half-life and uncertainty, branching ratio, decay Q; (2) decay radiation: for each nuclide, tables of radiation energy, intensity andmore » equivalent dose for the 5 most intense decay radiations of beta+, beta-, conversion electrons, gammas, alphas and x-rays, including electron Augers; (3) adopted gammas: for each nuclide, table containing energy, relative intensity, energy level of the main gamma lines and year of publication in Nuclear Data Sheets; (4) search gamma energies: for a specified interval of gamma energies all know gamma lines and their nuclides are displayed; the database contains 132,000 gamma lines; (5) a search mode by specific nuclide is also available. For the latest data and online tools for viewing the data, see NuDat 2.4 on the NNDC and IAEA NDS websites: http://www.nndc.bnl.gov/ and http://www-nds.iaea.org/.« less

  20. Scaling in situ cosmogenic nuclide production rates using analytical approximations to atmospheric cosmic-ray fluxes

    NASA Astrophysics Data System (ADS)

    Lifton, Nathaniel; Sato, Tatsuhiko; Dunai, Tibor J.

    2014-01-01

    Several models have been proposed for scaling in situ cosmogenic nuclide production rates from the relatively few sites where they have been measured to other sites of interest. Two main types of models are recognized: (1) those based on data from nuclear disintegrations in photographic emulsions combined with various neutron detectors, and (2) those based largely on neutron monitor data. However, stubborn discrepancies between these model types have led to frequent confusion when calculating surface exposure ages from production rates derived from the models. To help resolve these discrepancies and identify the sources of potential biases in each model, we have developed a new scaling model based on analytical approximations to modeled fluxes of the main atmospheric cosmic-ray particles responsible for in situ cosmogenic nuclide production. Both the analytical formulations and the Monte Carlo model fluxes on which they are based agree well with measured atmospheric fluxes of neutrons, protons, and muons, indicating they can serve as a robust estimate of the atmospheric cosmic-ray flux based on first principles. We are also using updated records for quantifying temporal and spatial variability in geomagnetic and solar modulation effects on the fluxes. A key advantage of this new model (herein termed LSD) over previous Monte Carlo models of cosmogenic nuclide production is that it allows for faster estimation of scaling factors based on time-varying geomagnetic and solar inputs. Comparing scaling predictions derived from the LSD model with those of previously published models suggest potential sources of bias in the latter can be largely attributed to two factors: different energy responses of the secondary neutron detectors used in developing the models, and different geomagnetic parameterizations. Given that the LSD model generates flux spectra for each cosmic-ray particle of interest, it is also relatively straightforward to generate nuclide-specific scaling

  1. A modified direct method for the calculation of elastic moduli of composite materials

    SciTech Connect

    Wang, J.A.; Lubliner, J.; Monteiro, P.J.M.

    1996-02-01

    The modified direct method is a scheme for the estimation of elastic moduli of composite materials and is based on micromechanical theory and classical elasticity. Using the statistical homogeneous assumption and the two-phase composite approach, one takes the average field of the composite. Due to the complexity of composite materials, the modeling parameters for the exact analytical theory are not always available and then the effective bounds are usually too wide for practical application. For engineering purposes a more practical and general model is desired. The modified direct method was developed to approach the above requirements. In this work the modified direct method is compared with different available experiment data and methods, for example, Kuster-Toksoez, Christensen-Lo. The comparison results show that the modified direct method provides a very good estimation of the elastic moduli in different kinds of problems, such as the soft and hard inclusion cases, porous materials, at various concentrations and/or various porosities.

  2. Calculation of the elastic properties of a triangular cell core for lightweight composite mirrors

    NASA Astrophysics Data System (ADS)

    Penado, F. Ernesto; Clark, James H., III; Walton, Joshua P.; Romeo, Robert C.; Martin, Robert N.

    2007-09-01

    The use of composite materials in the fabrication of optical telescope mirrors offers many advantages over conventional methods, including lightweight, portability and the potential for lower manufacturing costs. In the construction of the substrate for these mirrors, sandwich construction offers the advantage of even lower weight and higher stiffness. Generally, an aluminum or Nomex honeycomb core is used in composite applications requiring sandwich construction. However, the use of a composite core offers the potential for increased stiffness and strength, low thermal distortion compatible with that of the facesheets, the absence of galvanic corrosion and the ability to readily modify the core properties. In order to design, analyze and optimize these mirrors, knowledge of the mechanical properties of the core is essential. In this paper, the mechanical properties of a composite triangular cell core (often referred to as isogrid) are determined using finite element analysis of a representative unit cell. The core studied offers many advantages over conventional cores including increased thermal and dimensional stability, as well as low weight. Results are provided for the engineering elastic moduli of cores made of high stiffness composite material as a function of the ply layup and cell size. Finally, in order to illustrate the use of these properties in a typical application, a 1.4-m diameter composite mirror is analyzed using the finite element method, and the resulting stiffness and natural frequencies are presented.

  3. Initial Test Determination of Cosmogenic Nuclides in Magnetite

    NASA Astrophysics Data System (ADS)

    Matsumura, H.; Caffee, M. W.; Nagao, K.; Nishiizumi, K.

    2014-12-01

    Long-lived radionuclides, such as 10Be, 26Al, and 36Cl, are produced by cosmic rays in surficial materials on Earth, and used for determinations of cosmic-ray exposure ages and erosion rates. Quartz and limestone are routinely used as the target minerals for these geomorphological studies. Magnetite also contains target elements that produce abundant cosmogenic nuclides when exposed to the cosmic rays. Magnetite has several notable merits that enable the measurement of cosmogenic nuclides: (1) the target elements for production of cosmogenic nuclides in magnetite comprise the dominant mineral form of magnetite, Fe3O4; (2) magnetite can be easily isolated, using a magnet, after rock milling; (3) multiple cosmogenic nuclides are produced by exposure of magnetite to cosmic-ray secondaries; and (4) cosmogenic nuclides produced in the rock containing the magnetite, but not within the magnetite itself, can be separated using nitric acid and sodium hydroxide leaches. As part of this initial study, magnetite was separated from a basaltic sample collected from the Atacama Desert in Chili (2,995 m). Then Be, Al, Cl, Ca, and Mn were separated from ~2 g of the purified magnetite. We measured cosmogenic 10Be, 26Al, and 36Cl concentrations in the magnetite by accelerator mass spectrometry at PRIME Lab, Purdue University. Cosmogenic 3He and 21Ne concentrations of aliquot of the magnetite were measured by mass spectrometry at the University of Tokyo. We also measured the nuclide concentrations from magnetite collected from a mine at Ishpeming, Michigan as a blank. The 10Be and 36Cl concentrations as well as 3He concentration produce concordant cosmic ray exposure ages of ~0.4 Myr for the Atacama basalt. However, observed high 26Al and 21Ne concentrations attribute to those nuclides incorporation from silicate impurity.

  4. Development of an analytic procedure to calculate damage accumulation in composites during low velocity impact

    NASA Technical Reports Server (NTRS)

    Humphreys, E. A.; Goering, J.

    1983-01-01

    A computerized procedure was developed to model the response of a laminated composite plate subjected to low velocity impact. The methodology incorporated transient dynamics finite element analysis coupled with composite layer and interlaminar stress predictions. Damage was predicted using a stress based failure criteria and incorporated into the solution as stiffness modifications. The force-displacement relation between the impactor and plate was modelled with a nonlinear contact spring similar to Hertzian contact. Analyses performed predicted ply damage early in the impact event when the displacement fields were characteristic of high frequency flexurable response.

  5. Electron and proton absorption calculations for a graphite/epoxy composite model. [large space structures

    NASA Technical Reports Server (NTRS)

    Long, E. R., Jr.

    1979-01-01

    The Bethe-Bloch stopping power relations for inelastic collisions were used to determine the absorption of electron and proton energy in cured neat epoxy resin and the absorption of electron energy in a graphite/epoxy composite. Absorption of electron energy due to bremsstrahlung was determined. Electron energies from 0.2 to 4.0 MeV and proton energies from 0.3 to 1.75 MeV were used. Monoenergetic electron energy absorption profiles for models of pure graphite, cured neat epoxy resin, and graphite/epoxy composites are reported. A relation is determined for depth of uniform energy absorption in a composite as a function of fiber volume fraction and initial electron energy. Monoenergetic proton energy absorption profiles are reported for the neat resin model. A relation for total proton penetration in the epoxy resin as a function of initial proton energy is determined. Electron energy absorption in the composite due to bremsstrahlung is reported. Electron and proton energy absorption profiles in cured neat epoxy resin are reported for environments approximating geosynchronous earth orbit.

  6. 40 CFR 1066.820 - Composite calculations for FTP exhaust emissions.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... composite gaseous test results as a mass-weighted value, e -FTPcomp, in grams per mile using the following... interval (generally known as bag 1 and bag 2), in grams. D ct = the measured driving distance from the... from the hot-start UDDS test interval in grams. This is the hot-stabilized portion from either...

  7. Stress Free Temperature Testing and Calculations on Out-of-Autoclave Composites

    NASA Technical Reports Server (NTRS)

    Cox, Sarah B.; Tate, LeNetra C.; Danley, Susan E.; Sampson, Jeffrey W.; Taylor, Brian J.; Sutter, James K.; Miller, Sandi G.

    2013-01-01

    Future launch vehicles will require the incorporation of large composite parts that will make up primary and secondary components of the vehicle. NASA has explored the feasibility of manufacturing these large components using Out-of-Autoclave impregnated carbon fiber composite systems through many composites development projects. Most recently, the Composites for Exploration Project has been looking at the development of a 10 meter diameter fairing structure, similar in size to what will be required for a heavy launch vehicle. The development of new material systems requires the investigation of the material properties and the stress in the parts. Residual stress is an important factor to incorporate when modeling the stresses that a part is undergoing. Testing was performed to verify the stress free temperature with two-ply asymmetric panels. A comparison was done between three newly developed out of autoclave IM7/Bismaleimide (BMI) systems. This paper presents the testing results and the analysis performed to determine the stress free temperature of the materials

  8. Stress Free Temperature Testing and Residual Stress Calculations on Out-of-Autoclave Composites

    NASA Technical Reports Server (NTRS)

    Cox, Sarah; Tate, LaNetra C.; Danley, Susan; Sampson, Jeff; Taylor, Brian; Miller, Sandi

    2012-01-01

    Future launch vehicles will require the incorporation large composite parts that will make up primary and secondary components of the vehicle. NASA has explored the feasibility of manufacturing these large components using Out-of-Autoclave impregnated carbon fiber composite systems through many composites development projects. Most recently, the Composites for Exploration Project has been looking at the development of a 10 meter diameter fairing structure, similar in size to what will be required for a heavy launch vehicle. The development of new material systems requires the investigation of the material properties and the stress in the parts. Residual stress is an important factor to incorporate when modeling the stresses that a part is undergoing. Testing was performed to verify the stress free temperature with two-ply asymmetric panels. A comparison was done between three newly developed out of autoclave IM7 /Bismalieimide (BMI) systems. This paper presents the testing results and the analysis performed to determine the residual stress of the materials.

  9. Computer program for calculation of complex chemical equilibrium compositions and applications. Part 1: Analysis

    NASA Technical Reports Server (NTRS)

    Gordon, Sanford; Mcbride, Bonnie J.

    1994-01-01

    This report presents the latest in a number of versions of chemical equilibrium and applications programs developed at the NASA Lewis Research Center over more than 40 years. These programs have changed over the years to include additional features and improved calculation techniques and to take advantage of constantly improving computer capabilities. The minimization-of-free-energy approach to chemical equilibrium calculations has been used in all versions of the program since 1967. The two principal purposes of this report are presented in two parts. The first purpose, which is accomplished here in part 1, is to present in detail a number of topics of general interest in complex equilibrium calculations. These topics include mathematical analyses and techniques for obtaining chemical equilibrium; formulas for obtaining thermodynamic and transport mixture properties and thermodynamic derivatives; criteria for inclusion of condensed phases; calculations at a triple point; inclusion of ionized species; and various applications, such as constant-pressure or constant-volume combustion, rocket performance based on either a finite- or infinite-chamber-area model, shock wave calculations, and Chapman-Jouguet detonations. The second purpose of this report, to facilitate the use of the computer code, is accomplished in part 2, entitled 'Users Manual and Program Description'. Various aspects of the computer code are discussed, and a number of examples are given to illustrate its versatility.

  10. Variable temperature effects on release rates of readily soluble nuclides

    SciTech Connect

    Kim, C.-L.; Light, W.B.; Lee, W.W.-L.; Chambre, P.L.; Pigford, T.H.; Lawrence Berkeley Lab., CA )

    1988-09-01

    In this paper we study the effect of temperature on the release rate of readily soluble nuclides, as affected by a time-temperature dependent diffusion coefficient. In this analysis ground water fills the voids in the waste package at t = 0 and one percent of the inventories of cesium and iodine are immediately dissolved into the void water. Mass transfer resistance of partly failed container and cladding is conservatively neglected. The nuclides move through the void space into the surrounding rock under a concentration gradient. We use an analytic solution to compute the nuclide concentration in the gap or void, and the mass flux rate into the porous rock. 8 refs., 4 figs.

  11. rp Process and Masses of N{approx_equal}Z{approx_equal}34 Nuclides

    SciTech Connect

    Savory, J.; Schury, P.; Bachelet, C.; Block, M.; Bollen, G.; Facina, M.; Folden, C. M. III; Guenaut, C.; Kwan, E.; Kwiatkowski, A. A.; Morrissey, D. J.; Pang, G. K.; Prinke, A.; Ringle, R.; Schatz, H.; Schwarz, S.; Sumithrarachchi, C. S.

    2009-04-03

    High-precision Penning-trap mass measurements of the N{approx_equal}Z{approx_equal}34 nuclides {sup 68}Se, {sup 70}Se, {sup 70m}Br, and {sup 71}Br were performed, reaching experimental uncertainties of 0.5-15 keV. The new and improved mass data together with theoretical Coulomb displacement energies were used as input for rp process network calculations. An increase in the effective lifetime of the waiting point nucleus {sup 68}Se was found, and more precise information was obtained on the luminosity during a type I x-ray burst along with the final elemental abundances after the burst.

  12. Calculating the performance of 1{endash}3 piezoelectric composites for hydrophone applications: An effective medium approach

    SciTech Connect

    Avellaneda, M.; Swart, P.J.

    1998-03-01

    A new method is presented for evaluating the performance of 1{endash}3 polymer/piezoelectric ceramic composites for hydrophone applications. The Poisson`s ratio effect, i.e., the enhancement of the hydrostatic performance which can be achieved by mixing piezoelectric ceramics with polymers, is studied in detail. Using an `effective medium` approach, algebraic expressions are derived for the composite hydrostatic charge coefficient d{sub h}, the hydrostatic figure of merit d{sub h}g{sub h}, and the hydrostatic electromechanical coupling coefficient k{sub h} in terms of the properties of the constituent materials, the ceramic volume fraction, and a microstructural parameter p. The high contrast in stiffness and dielectric constants existing between the two phases can be exploited to derive simple, geometry-independent approximations which explain quantitatively the Poisson`s ratio effect. It is demonstrated that the stiffness and the Poisson`s ratio of the polymer matrix play a crucial role in enhancing hydrophone performance. Using a differential scheme to model the parameter p, we evaluate d{sub h}, d{sub h}g{sub h}, and k{sub h} for polymer/piezoelectric ceramic systems at varying compositions. Several examples involving Pb(Zr,Ti)O{sub 3} and (Pb,Ca)TiO{sub 3} piezoelectric ceramics are given to illustrate the theory. {copyright} {ital 1998 Acoustical Society of America.}

  13. Computer program for calculation of complex chemical equilibrium compositions and applications. Supplement 1: Transport properties

    NASA Technical Reports Server (NTRS)

    Gordon, S.; Mcbride, B.; Zeleznik, F. J.

    1984-01-01

    An addition to the computer program of NASA SP-273 is given that permits transport property calculations for the gaseous phase. Approximate mixture formulas are used to obtain viscosity and frozen thermal conductivity. Reaction thermal conductivity is obtained by the same method as in NASA TN D-7056. Transport properties for 154 gaseous species were selected for use with the program.

  14. Study of interaction between radioactive nuclides and graphite surface by the first-principles and statistic physics

    NASA Astrophysics Data System (ADS)

    Luo, Xiaofeng; Fang, Chao; Li, Xin; Lai, Wensheng; Sun, Lifeng; Liang, Tongxiang

    2013-11-01

    The adsorption and desorption of four kinds of main radioactive productions (cesium, iodine, strontium and silver) on graphite surface in high temperature gas cooled reactors (HTGRs) have been studied. Using the first-principles density-functional theory, adsorptive geometry, energy and electron structure on the perfect and defective graphite surfaces have been calculated. It turns out that the adsorption of Cs, I and Sr atoms belongs to chemisorption while the adsorption of Ag is a pure physisorption. When introducing a vacancy in graphite surface, nuclide adatoms will be trapped by the vacancy and form chemical bonds with three nearest neighbor carbon atoms, leading to significant increase of the adsorption energy. In addition, a model of grand canonical ensemble is employed to deduce the adsorption rate as a function of temperature and partial pressure of nuclides produced. The transition temperate from adsorption to desorption of nuclides on graphite surface is defined as the inflexion point of the adsorption rate and its variation with nuclide density is obtained.

  15. An Approach to Calculate Mineralś Bulk Moduli KS from Chemical Composition and Density ρ

    NASA Astrophysics Data System (ADS)

    Breuer, S.; Schilling, F. R.; Mueller, B.; Drüppel, K.

    2015-12-01

    The elastic properties of minerals are fundamental parameters for technical and geotechnical applications and an important research topic towards a better understanding of the Eart&hacute;s interior. Published elastic properties, chemical composition, and density data of 86 minerals (total of 258 data including properties of minerals at various p, T conditions) were collected into a database. It was used to test different hypotheses about relationships between these properties (e.g. water content in minerals and their Poisson's ratio). Furthermore, a scheme to model the average elastic properties, i.e. the bulk modulus KS, based on mineral density and composition was developed. Birc&hacute;s law, a linearity between density ρ and wave velocity (e.g. vp.), is frequently used in seismic and seismology to derive density of the Eart&hacute;s interior from seismic velocities. Applying the compiled mineral data contradicts the use of a simple velocity-density relation (e.g. Gardneŕs relation, 1974). The presented model-approach to estimate the mineralś bulk moduli Ks (as Voigt-Reuss-Hill average) is based on the idea of pressure-temperature (p-T) dependent ionś bulk moduli. Using a multi-exponential regression to ascertain the ionś bulk moduli and by applying an exponential scaling with density ρ, their bulk moduli could be modelled. As a result, > 88 % of the 258 bulk moduli data are predicted with an uncertainty of < 20 % compared to published values. Compared to other models (e.g. Anderson et al. 1970 and Anderson & Nafe 1965), the here presented approach to model the bulk moduli only requires the density ρ and chemical composition of the mineral and is not limited to a specific group of minerals, composition, or structure. In addition to this, by using the pressure and temperature dependent density ρ(p, T), it is possible to predict bulk moduli for varying p-T conditions. References:Gardner, G.H.F, Gardner, L.W. and Gregory, A.R. (1974). Geophysics, 39, No. 6

  16. An Approach to Calculate Mineralś Bulk Moduli KS from Chemical Composition and Density ρ

    NASA Astrophysics Data System (ADS)

    Breuer, S.; Schilling, F. R.; Mueller, B.; Drüppel, K.

    2015-12-01

    The elastic properties of minerals are fundamental parameters for technical and geotechnical applications and an important research topic towards a better understanding of the Earth's interior. Published elastic properties, chemical composition, and density data of 86 minerals (total of 258 data including properties of minerals at various p, T conditions) were collected into a database. It was used to test different hypotheses about relationships between these properties (e.g. water content in minerals and their Poisson's ratio). Furthermore, a scheme to model the average elastic properties, i.e. the bulk modulus KS, based on mineral density and composition was developed. Birch's law, a linearity between density ρ and wave velocity (e.g. vp.), is frequently used in seismic and seismology to derive density of the Earth's interior from seismic velocities. Applying the compiled mineral data contradicts the use of a simple velocity-density relation (e.g. Gardneŕs relation, 1974). The presented model-approach to estimate the mineralś bulk moduli Ks (as Voigt-Reuss-Hill average) is based on the idea of pressure-temperature (p-T) dependent ionś bulk moduli. Using a multi-exponential regression to ascertain the ionś bulk moduli and by applying an exponential scaling with density ρ, their bulk moduli could be modelled. As a result, > 88 % of the 258 bulk moduli data are predicted with an uncertainty of < 20 % compared to published values. Compared to other models (e.g. Anderson et al. 1970 and Anderson & Nafe 1965), the here presented approach to model the bulk moduli only requires the density ρ and chemical composition of the mineral and is not limited to a specific group of minerals, composition, or structure. In addition to this, by using the pressure and temperature dependent density ρ(p, T), it is possible to predict bulk moduli for varying p-T conditions. References:Gardner, G.H.F, Gardner, L.W. and Gregory, A.R. (1974). Geophysics, 39, No. 6, 770

  17. Chemical composition data and calculated aquifer temperature for selected wells and springs of Honey Lake Valley, California

    USGS Publications Warehouse

    Mariner, R.H.; Presser, T.S.; Evans, William C.

    1976-01-01

    Major element, minor element, and gas composition data are tabulated for 15 springs and wells in Honey Lake Valley, California. Wendel and Amedee hot springs issue Na-S04-C1 waters at boiling or near boiling temperatures; the remaining springs and wells issue Na-HC03 waters at temperatures ranging from 14 to 33 deg C. Gases escaping from the hot springs are principally nitrogen with minor amounts of methane. The geothermometers calculated from the chemical data are also tabulated for each spring. (Woodard-USGS)

  18. Electronic interaction in composites of a conjugated polymer and carbon nanotubes: first-principles calculation and photophysical approaches

    PubMed Central

    Wéry, Jany; Duvail, Jean-Luc; Lefrant, Serge; Yaya, Abu; Ewels, Chris

    2015-01-01

    Summary The mechanisms that control the photophysics of composite films made of a semiconducting conjugated polymer (poly(paraphenylene vinylene), PPV) mixed with single-walled carbon nanotubes (SWNT) up to a concentration of 64 wt % are determined by using photoexcitation techniques and density functional theory. Charge separation is confirmed experimentally by rapid quenching of PPV photoluminescence and changes in photocurrent starting at relatively low concentrations of SWNT. Calculations predict strong electronic interaction between the polymer and the SWNT network when nanotubes are semiconducting. PMID:26171290

  19. A Novel Method for Calculation of Strain Energy Release Rate of Asymmetric Double Cantilever Laminated Composite Beams

    NASA Astrophysics Data System (ADS)

    Shokrieh, M. M.; Zeinedini, A.

    2014-06-01

    In this research, a novel data reduction method for calculation of the strain energy release rate ( SERR) of asymmetric double cantilever beams ( ADCB) is presented. For this purpose the elastic beam theory ( EBT) is modified and the new method is called as the modified elastic beam theory ( MEBT). Also, the ADCB specimens are modeled using ABAQUS/Standard software. Then, the initiation of delamination of ADCB specimens is modeled using the virtual crack closure technique ( VCCT). Furthermore, magnitudes of the SERR for different samples are also calculated by an available data reduction method, called modified beam theory ( MBT). Using the hand lay-up method, different laminated composite samples are manufactured by E-glass/epoxy unidirectional plies. In order to measure the SERR, all samples are tested using an experimental setup. The results determined by the new data reduction method ( MEBT) show good agreements with the results of the VCCT and the MBT.

  20. Theoretical calculation of a composite pulse for 2H broadband excitation by average Hamiltonian theory

    PubMed Central

    Shen, Ming; Roopchand, Rabia; Amoureux, Jean-Paul; Chen, Qun

    2015-01-01

    Quadrupolar echo NMR spectroscopy of solids often requires RF pulse excitation that covers spectral widths exceeding 100 kHz. In a recent work we found out that a four pulse, composite pulse COM-II ( 90180¯90135¯45 ), provided robust broadband excitation for deuterium quadrupolar echo spectroscopy. Moreover, when combined with an eight step phase cycle, spectral distortions arising from finite pulse widths were greatly supressed. In this paper we report on a theoretical analysis COM-II with 8-step phase cycle by average Hamiltonian theory. This treatment is combined with the fictitious spin-1 operator formalism, and the mechanism of the 8-step phase cycling that minimizes the spectral distortions is discussed. PMID:26681896

  1. Calculation of skin-stiffener interface stresses in stiffened composite panels

    NASA Technical Reports Server (NTRS)

    Cohen, David; Hyer, Michael W.

    1987-01-01

    A method for computing the skin-stiffener interface stresses in stiffened composite panels is developed. Both geometrically linear and nonlinear analyses are considered. Particular attention is given to the flange termination region where stresses are expected to exhibit unbounded characteristics. The method is based on a finite-element analysis and an elasticity solution. The finite-element analysis is standard, while the elasticity solution is based on an eigenvalue expansion of the stress functions. The eigenvalue expansion is assumed to be valid in the local flange termination region and is coupled with the finite-element analysis using collocation of stresses on the local region boundaries. Accuracy and convergence of the local elasticity solution are assessed using a geometrically linear analysis. Using this analysis procedure, the influence of geometric nonlinearities and stiffener parameters on the skin-stiffener interface stresses is evaluated.

  2. Mid-Pleistocene cosmogenic minimum-age limits for pre-Wisconsinan glacial surfaces in southwestern Minnesota and southern Baffin Island: A multiple nuclide approach

    USGS Publications Warehouse

    Bierman, P.R.; Marsella, K.A.; Patterson, Chris; Davis, P.T.; Caffee, M.

    1999-01-01

    Paired 10Be and 26Al analyses (n = 14) indicate that pre-Wisconsinan, glaciated bedrock surfaces near the northern (Baffin Island) and southern (Minnesota) paleo-margins of the Laurentide Ice Sheet have long and complex histories of cosmic-ray exposure, including significant periods of partial or complete shielding from cosmic rays. Using the ratio, 26Al/10Be, we calculate that striated outcrops of Sioux Quartzite in southwestern Minnesota (southern margin) were last overrun by ice at least 500,000 years ago. Weathered bedrock tors on the once-glaciated uplands of Baffin Island (northern margin) are eroding no faster than 1.1 m Myr-1, the equivalent of at least 450,000 years of surface and near-surface exposure. Our data demonstrate that exposure ages and erosion rates calculated from single nuclides can underestimate surface stability dramatically because any intermittent burial, and the resultant lowering of nuclide production rates and nuclide abundances, will remain undetected.

  3. Cosmogenic neutron-capture-produced nuclides in stony meteorites

    NASA Technical Reports Server (NTRS)

    Spergel, M. S.; Reedy, R. C.; Lazareth, O. W.; Levy, P. W.; Slatest, L. A.

    1986-01-01

    The complete neutron-flux results and production rates for Cl-36, Ni-59, and Co-60 in stony meteorites of various radii and composition are presented. The relative neutron source strengths and neutron production-versus-depth profiles were determined by using calculated H-3 production rates. The absolute source strengths were normalized to that determined for the moon by Woolum et al. (1975). The energy spectrum of the source neutrons and the neutron transport calculations, which employed the ANISN computer code, were similar to those used for the moon by Lingenfelter et al. (1972). The production rates of the three radionuclides were determined as a function of depth in various spherical meteoroids from the calculated equilibrium neutron-flux distributions and from energy-dependent neutron-capture cross sections. Rates for producing these radionuclides by spallation reactions were also calculated.

  4. Dependence of nuclear quadrupole resonance transitions on the electric field gradient asymmetry parameter for nuclides with half-integer spins

    NASA Astrophysics Data System (ADS)

    Cho, Herman

    2016-09-01

    Allowed transition energies and eigenstate expansions have been calculated and tabulated in numerical form as functions of the electric field gradient asymmetry parameter for the zero field Hamiltonian of quadrupolar nuclides with I = 3 / 2 , 5 / 2 , 7 / 2, and 9 / 2. These results are essential to interpret nuclear quadrupole resonance (NQR) spectra and extract accurate values of the electric field gradient tensors. Applications of NQR methods to studies of electronic structure in heavy element systems are proposed.

  5. Dependence of nuclear quadrupole resonance transitions on the electric field gradient asymmetry parameter for nuclides with half-integer spins

    DOE PAGESBeta

    Cho, Herman

    2016-02-28

    Allowed transition energies and eigenstate expansions have been calculated and tabulated in numerical form as functions of the electric field gradient asymmetry parameter for the zero field Hamiltonian of quadrupolar nuclides with I = 3/2,5/2,7/2, and 9/2. These results are essential to interpret nuclear quadrupole resonance (NQR) spectra and extract accurate values of the electric field gradient tensors. Furthermore, applications of NQR methods to studies of electronic structure in heavy element systems are proposed.

  6. Comparison of measured and calculated composition of irradiated EBR-II blanket assemblies.

    SciTech Connect

    Grimm, K. N.

    1998-07-13

    In anticipation of processing irradiated EBR-II depleted uranium blanket subassemblies in the Fuel Conditioning Facility (FCF) at ANL-West, it has been possible to obtain a limited set of destructive chemical analyses of samples from a single EBR-II blanket subassembly. Comparison of calculated values with these measurements is being used to validate a depletion methodology based on a limited number of generic models of EBR-II to simulate the irradiation history of these subassemblies. Initial comparisons indicate these methods are adequate to meet the operations and material control and accountancy (MC and A) requirements for the FCF, but also indicate several shortcomings which may be corrected or improved.

  7. An Analytical Investigation of Three General Methods of Calculating Chemical-Equilibrium Compositions

    NASA Technical Reports Server (NTRS)

    Zeleznik, Frank J.; Gordon, Sanford

    1960-01-01

    The Brinkley, Huff, and White methods for chemical-equilibrium calculations were modified and extended in order to permit an analytical comparison. The extended forms of these methods permit condensed species as reaction products, include temperature as a variable in the iteration, and permit arbitrary estimates for the variables. It is analytically shown that the three extended methods can be placed in a form that is independent of components. In this form the Brinkley iteration is identical computationally to the White method, while the modified Huff method differs only'slightly from these two. The convergence rates of the modified Brinkley and White methods are identical; and, further, all three methods are guaranteed to converge and will ultimately converge quadratically. It is concluded that no one of the three methods offers any significant computational advantages over the other two.

  8. Shielding and activity estimator for template-based nuclide identification methods

    DOEpatents

    Nelson, Karl Einar

    2013-04-09

    According to one embodiment, a method for estimating an activity of one or more radio-nuclides includes receiving one or more templates, the one or more templates corresponding to one or more radio-nuclides which contribute to a probable solution, receiving one or more weighting factors, each weighting factor representing a contribution of one radio-nuclide to the probable solution, computing an effective areal density for each of the one more radio-nuclides, computing an effective atomic number (Z) for each of the one more radio-nuclides, computing an effective metric for each of the one or more radio-nuclides, and computing an estimated activity for each of the one or more radio-nuclides. In other embodiments, computer program products, systems, and other methods are presented for estimating an activity of one or more radio-nuclides.

  9. Fuel Thermo-physical Characterization Project: Evaluation of Models to Calculate Thermal Diffusivity of Layered Composites

    SciTech Connect

    Burkes, Douglas; Casella, Amanda J.; Gardner, Levi D.; Casella, Andrew M.; Huber, Tanja K.; Breitkreutz, Harald

    2015-02-11

    The Office of Material Management and Minimization Fuel Thermo-physical Characterization Project at Pacific Northwest National Laboratory (PNNL) is tasked with using PNNL facilities and processes to receive irradiated low enriched uranium-molybdenum fuel plate samples and perform analyses in support of the Office of Material Management and Minimization Reactor Conversion Program. This work is in support of the Fuel Development Pillar that is managed by Idaho National Laboratory. A key portion of the scope associated with this project was to measure the thermal properties of fuel segments harvested from plates that were irradiated in the Advanced Test Reactor. Thermal diffusivity of samples prepared from the fuel segments was measured using laser flash analysis. Two models, one developed by PNNL and the other developed by the Technische Universität München (TUM), were evaluated to extract the thermal diffusivity of the uranium-molybdenum alloy from measurements made on the irradiated, layered composites. The experimental data of the “TC” irradiated fuel segment was evaluated using both models considering a three-layer and five-layer system. Both models are in acceptable agreement with one another and indicate that the zirconium diffusion barrier has a minimal impact on the overall thermal diffusivity of the monolithic U-Mo fuel.

  10. Theoretical Investigation of Calculating Temperatures in the Combining Zone of Cu/Fe Composite Plate Jointed by Explosive Welding

    NASA Astrophysics Data System (ADS)

    Qu, Y. D.; Zhang, W. J.; Kong, X. Q.; Zhao, X.

    2016-03-01

    The heat-transfer behavior of the interface of Flyer plate (or Base Plate) has great influence on the microcosmic structures, stress distributions, and interface distortion of the welded interface of composite plates by explosive welding. In this paper, the temperature distributions in the combing zone are studied for the case of Cu/Fe composite plate jointed by explosive welding near the lower limit of explosive welding. The results show that Flyer plate (Cu plate) and Base Plate (Fe plate) firstly almost have the same melting rate in the explosive welding process. Then, the melting rate of Cu plate becomes higher than that of Fe plate. Finally, the melt thicknesses of Cu plate and Fe plate trend to be different constants, respectively. Meanwhile, the melting layer of Cu plate is thicker than that of Fe plate. The research could supply some theoretical foundations for calculating the temperature distribution and optimizing the explosive welding parameters of Cu/Fe composite plate to some extent.

  11. Constraints on Abundances and Compositional Ranges of X-Ray Amorphous Components in Soils and Rocks at Gale Crater from Mass Balance Calculations

    NASA Astrophysics Data System (ADS)

    Dehouck, E.; McLennan, S. M.; Meslin, P.-Y.; Cousin, A.; Rampe, E. B.; Morris, R. V.; Lanza, N. L.; Hurowitz, J. A.; Rapin, W.; MSL Science Team

    2014-07-01

    We present the results of mass balance calculations that explore the domain of possible chemical compositions (with constraints on abundances) of the amorphous component detected by Curiosity within the Rocknest and Cumberland samples.

  12. Calculation of optical properties of dental composites as a basis for determining color impression and penetration depth of laser light

    NASA Astrophysics Data System (ADS)

    Weniger, Kirsten K.; Muller, Gerhard J.

    2005-03-01

    In order to achieve esthetic dental restorations, there should be no visible difference between restorative material and treated teeth. This requires a match of the optical properties of both restorative material and natural teeth. These optical properties are determined by absorption and scattering of light emerging not only on the surface but also inside the material. Investigating different dental composites in several shades, a method has been developed to calculate the optical parameters absorption coefficient μa, scattering coefficient μs, anisotropy factor g and reduced scattering coefficient μs'. The method includes sample preparation and measurements of transmittance and reflectance in an integrating sphere spectrometer, followed by inverse Monte Carlo simulations. Determination of optical properties is more precise and comprehensive than with the previously used Kubelka Munk theory because scattering can be looked at separated into pure scattering with the scattering coefficient μs and its direction with the anisotropy factor g. Moreover the use of the inverse Monte Carlo simulation not only minimizes systematic errors and considers the scattering phase function, but also takes into account the measuring geometry. The compilation of a data pool of optical parameters now enables the application of further calculation models as a basis for optimization of the composition of new materials. For example, a prediction of the general color impression for multiple layers can be carried out as well as the calculation of the wavelength dependent penetration depths of light with regard to photo polymerization. Further applications are possible in the area of laser ablation.

  13. Regular Cosmogenic Nuclide Dosing of Sediment Moving Down Desert Piedmonts

    NASA Astrophysics Data System (ADS)

    Nichols, K. K.; Bierman, P. R.; Hooke, R. L.; Eppes, M. C.; Persico, L.; Caffee, M.; Finkel, R.

    2001-12-01

    Low-gradient alluvial piedmonts are common in desert areas throughout the world; however, long-term rates of processes that modify these landscapes are poorly understood. Using cosmogenic 10Be and 26Al, we attempt to quantify the long-term (>103 y) behavior of desert piedmonts in Southern California. We measured the activity of 10Be and 26Al in three samples of drainage basin alluvium and six amalgamated samples from transects spaced at 1-km intervals down a piedmont in Fort Irwin, Mojave Desert, California. Each transect sample consists of sediment from 21 collection sites spaced at 150 m intervals. Such sampling averages the variability of nuclide activity between sub-sample locations and thus gives a long-term dosing history of sediment as it is transported from uplands to the distal piedmont. The piedmont is heavily used during military training exercises during which hundreds of wheeled and tracked vehicles traverse the surface. The piedmont surface is planar, and fan-head incision is minimal at the rangefront decreasing to zero between the first and second transects, 1.5 km from the rangefront. 10Be activity increases steadily from 5.87 X 105 atoms g-1 at the rangefront to 1.02 X 6 atoms g-1 at the piedmont bottom. Nuclide activity and distance are well correlated (r2 = 0.95) suggesting that sediment is dosed uniformly as it is transported down piedmont. We have measured similar increases in nuclide activity in transect samples collected from two other Mojave Desert piedmonts, those fringing the Iron and Granite Mountains (Nichols et al, in press, Geomorphology). These piedmonts have nuclide activities that also correlate well with distance (r2 = 0.98 and 0.96, respectively) from their rangefronts, but nuclides increase at a lower rate down piedmont. Modeled sediment transport speeds for the Iron and Granite Mountain piedmonts are decimeters per year. The regular increase in nuclide activities down three different Mojave Desert piedmonts suggests that

  14. Sand residence times of one million years in the Namib Sand Sea from cosmogenic nuclides

    NASA Astrophysics Data System (ADS)

    Vermeesch, P.; Fenton, C. R.; Kober, F.; Wiggs, G. F. S.; Bristow, C. S.; Xu, S.

    2010-12-01

    The Namib Sand Sea is one of the world's oldest and largest sand deserts, yet little is known about the source of the sand in this, or other large deserts. In particular, it is unclear whether the sand is derived from local sediment or comes from remote sources. The relatively uniform appearance of dune sands and low compositional variability within dune fields make it difficult to address this question. Here we combine cosmogenic-nuclide measurements and geochronological techniques to assess the provenance and migration history of sand grains in the Namib Sand Sea. We use U-Pb geochronology of detrital zircons to show that the primary source of sand is the Orange River at the southern edge of the Namib desert. Our burial ages obtained from measurements of the cosmogenic nuclides 10Be, 26Al and 21Ne suggest that the residence time of sand within the sand sea is at least one million years. We therefore conclude that, despite large climatic changes in the Namib region associated with Quaternary glacial-interglacial cycles, the area currently occupied by the Namib Sand Sea has never been entirely devoid of sand during the past million years.

  15. Radio-nuclide mixture identification using medium energy resolution detectors

    SciTech Connect

    Nelson, Karl Einar

    2013-09-17

    According to one embodiment, a method for identifying radio-nuclides includes receiving spectral data, extracting a feature set from the spectral data comparable to a plurality of templates in a template library, and using a branch and bound method to determine a probable template match based on the feature set and templates in the template library. In another embodiment, a device for identifying unknown radio-nuclides includes a processor, a multi-channel analyzer, and a memory operatively coupled to the processor, the memory having computer readable code stored thereon. The computer readable code is configured, when executed by the processor, to receive spectral data, to extract a feature set from the spectral data comparable to a plurality of templates in a template library, and to use a branch and bound method to determine a probable template match based on the feature set and templates in the template library.

  16. Recent MARS15 developments: nuclide inventory, DPA and gas production

    SciTech Connect

    Mokhov, N.V.; /Fermilab

    2010-12-01

    Recent developments in the MARS15 code are described for the critical modules related to demands of hadron and lepton colliders and Megawatt proton and heavy-ion beam facilities. Details of advanced models for particle production and nuclide distributions in nuclear interactions at low and medium energies, energy loss, atomic displacements and gas production are presented along with benchmarking against data. Recent developments in the MARS15 physics models, such as nuclide production, decay and transmutation and all-component DPA modelling for arbitrary projectiles in the 1 keV to 10 TeV energy range, add new capabilities to the code crucial in numerous applications with high-intensity high-power beams. Some discrepancies in DPA rate predictions by several codes, relation of DPA and H/He production rates to changes in material properties, as well as corresponding experimental studies at energies above a hundred of MeV are the areas requiring further efforts.

  17. Measurements of cosmogenic nuclides in lunar rock 64455

    NASA Technical Reports Server (NTRS)

    Arnold, J. R.; Kohl, C. P.; Nishiizumi, K.; Caffee, M. W.; Finkel, R. C.; Southon, J. R.

    1993-01-01

    Eleven samples were ground from the glass coated surface of lunar rock 64455,82 with an average depth resolution of 50 microns and were measured for Be-10, Al-26, and Cl-36 using AMS (accelerator mass spectrometry). Results show no evidence of SCR (solar cosmic ray) effects. The flat cosmogenic nuclide profiles and activity levels are consistent with a 2 My exposure history for the rock and a sample location on the bottom of the rock. These AMS measurements are some of the most precise ever obtained for these three nuclides. This precision and the demonstrated fine depth resolution will enable us to conduct a number of detailed studies of depth effects in lunar and meteoritic samples, including investigating SCR effects in the surface exposed top of the glass coating of 64455 and possibly in the underlying rock.

  18. Production rates of terrestrial in-situ-produced cosmogenic nuclides

    SciTech Connect

    Reedy, R.C.; Tuniz, C.; Fink, D.

    1993-12-31

    Production rates of cosmogenic nuclides made in situ in terrestrial samples and how they are applied to the interpretation of measured radionuclide concentrations were discussed at a one-day Workshop held 2 October 1993 in Sydney, Australia. The status of terrestrial in-situ studies using the long-lived radionuclides {sup 10}Be, {sup 14}C, {sup 26}Al, {sup 36}Cl, and {sup 41}Ca and of various modeling and related studies were presented. The relative uncertainties in the various factors that go into the interpretation of these terrestrial in-situ cosmogenic nuclides were discussed. The magnitudes of the errors for these factors were estimated and none dominated the final uncertainty.

  19. Hot demonstration of proposed commercial nuclide removal technology

    SciTech Connect

    Lee, D.

    1996-10-01

    This task covers the development and operation of an experimental test unit located in a Building 4501 hot cell within Building 4501 at Oak Ridge National Laboratory (ORNL). This equipment is designed to test radionuclides removal technologies under continuous operatoin on actual ORNL Melton Valley Storage Tank (MVST) supernatant, Savannah River high-level waste supernatant, and Hanford supernatant. The latter two may be simulated by adding the appropriate chemicals and/or nuclides to the MVST supernatant.

  20. A comparison of finite-difference and finite-element methods for calculating free edge stresses in composites

    NASA Technical Reports Server (NTRS)

    Bauld, N. R., Jr.; Goree, J. G.; Tzeng, L.-S.

    1985-01-01

    It is pointed out that edge delamination is a serious failure mechanism for laminated composite materials. Various numerical methods have been utilized in attempts to calculate the interlaminar stress components which precede delamination in a laminate. There are, however, discrepancies regarding the results provided by different methods, taking into account a finite-difference procedure, a perturbation procedure, and finite element approaches. The present investigation has the objective to assess the capacity of a finite difference method to predict the character and magnitude of the interlaminar stress distributions near an interface corner. A second purpose of the investigation is to determine if predictions by finite element method in-plane, interlaminar stress components near an interface corner represent actual laminate behavior.

  1. Atomic Mass Measurements of Stable and Unstable Nuclides

    NASA Astrophysics Data System (ADS)

    Dyck, Gary Robert

    1990-01-01

    This work describes three experiments in which precise atomic mass differences are determined by the technique of high resolution mass spectrometry. The Manitoba II mass spectrometer has been used to measure precise differences, involving naturally occurring nuclides, in two distinct studies, both of which have implications for the current work related to the question of neutrino mass. The first is a set of 6 doublet measurements in the Gd-Tb region, which show that the decay energy of 1220.64 +/- 0.83 keV is insufficient to allow the K-capture decay of ^{158} Tb to the 1187 keV level of ^{158 }Gd, which was proposed as a possible candidate for low energy beta decay in which the effect of a nu mass would be clearly seen. The second study is one in which 4 doublet spacings were determined in order to provide precise Q_ {2beta} values for the decays of ^{130}Te and ^{128}Te, which have long been of interest because they represent similar decays where the Q-values are significantly different. In a third experiment the Chalk River on-line isotope separator (ISOL) has been used to determine the masses of unstable nuclides. The tandem Van de Graaff accelerator was used to produce ^{105 }In, ^{104}In and ^{103}In which were then studied with the ISOL. This represents only the second time that masses of nuclides far from stability, other than alkali metals, have been determined directly.

  2. Recent developments in cosmogenic nuclide production rate scaling

    NASA Astrophysics Data System (ADS)

    Lifton, N. A.

    2013-12-01

    A new cosmogenic nuclide production rate scaling model based on analytical fits to Monte Carlo simulations of atmospheric cosmic ray flux spectra (both of which agree well with measured spectra) enables identification and quantification of the biases in previously published models (Lifton, N., Sato, T., Dunai, T., in review, Earth and Planet. Sci. Lett.). Scaling predictions derived from the new model (termed LSD) suggest two potential sources of bias in the previous models: different energy responses of the secondary neutron detectors used in developing the models, and different geomagnetic parameterizations. In addition, the particle flux spectra generated by the LSD model allow one to generate nuclide-specific scaling factors that reflect the influences of the flux energy distribution and the relevant excitation functions (probability of nuclide production in a given nuclear reaction as a function of energy). Resulting scaling factors indicate 3He shows the strongest positive deviation from the flux-based scaling, while 14C exhibits a negative deviation. These results are consistent with previous studies showing an increasing 3He/10Be ratio with altitude in the Himalayas, but with a much lower magnitude for the effect. Furthermore, the new model provides a flexible framework for exploring the implications of future advances in model inputs. For example, the effects of recently updated paleomagnetic models (e.g. Korte et al., 2011, Earth and Planet Sci. Lett. 312, 497-505) on scaling predictions will also be presented.

  3. Identification of heavy and superheavy nuclides using chemical separator systems

    NASA Astrophysics Data System (ADS)

    Türler, Andreas

    1999-11-01

    With the recent synthesis of superheavy nuclides produced in the reactions 48Ca+238U and 48Ca+242,244Pu, much longer-lived nuclei than the previously known neutron-deficient isotopes of the heaviest elements have been identified. Half-lives of several hours and up to several years have been predicted for the longest-lived isotopes of these elements. Thus, the sensitivity of radiochemical separation techniques may present a viable alternative to physical separator systems for the discovery of some of the predicted longer-lived heavy and superheavy nuclides. The advantages of chemical separator systems in comparison to kinematic separators lie in the possibility of using thick targets, high beam intensities spread over larger target areas and in providing access to nuclides emitted under large angles and low velocities. Thus, chemical separator systems are ideally suited to study also transfer and (HI, αxn) reaction products. In the following, a study of (HI, αxn) reactions will be presented and prospects to chemically identify heavy and superheavy elements discussed.

  4. Uncertainty in nutrient loads from tile-drained landscapes: Effect of sampling frequency, calculation algorithm, and compositing strategy

    NASA Astrophysics Data System (ADS)

    Williams, Mark R.; King, Kevin W.; Macrae, Merrin L.; Ford, William; Van Esbroeck, Chris; Brunke, Richard I.; English, Michael C.; Schiff, Sherry L.

    2015-11-01

    Accurate estimates of annual nutrient loads are required to evaluate trends in water quality following changes in land use or management and to calibrate and validate water quality models. While much emphasis has been placed on understanding the uncertainty of nutrient load estimates in large, naturally drained watersheds, few studies have focused on tile-drained fields and small tile-drained headwater watersheds. The objective of this study was to quantify uncertainty in annual dissolved reactive phosphorus (DRP) and nitrate-nitrogen (NO3-N) load estimates from four tile-drained fields and two small tile-drained headwater watersheds in Ohio, USA and Ontario, Canada. High temporal resolution datasets of discharge (10-30 min) and nutrient concentration (2 h to 1 d) were collected over a 1-2 year period at each site and used to calculate a reference nutrient load. Monte Carlo simulations were used to subsample the measured data to assess the effects of sample frequency, calculation algorithm, and compositing strategy on the uncertainty of load estimates. Results showed that uncertainty in annual DRP and NO3-N load estimates was influenced by both the sampling interval and the load estimation algorithm. Uncertainty in annual nutrient load estimates increased with increasing sampling interval for all of the load estimation algorithms tested. Continuous discharge measurements and linear interpolation of nutrient concentrations yielded the least amount of uncertainty, but still tended to underestimate the reference load. Compositing strategies generally improved the precision of load estimates compared to discrete grab samples; however, they often reduced the accuracy. Based on the results of this study, we recommended that nutrient concentration be measured every 13-26 h for DRP and every 2.7-17.5 d for NO3-N in tile-drained fields and small tile-drained headwater watersheds to accurately (±10%) estimate annual loads.

  5. Light-ion-induced reactions in mass measurements of neutron-deficient nuclides close to A = 100

    NASA Astrophysics Data System (ADS)

    Elomaa, V.-V.; Eronen, T.; Hager, U.; Hakala, J.; Jokinen, A.; Kankainen, A.; Moore, I. D.; Rahaman, S.; Rissanen, J.; Rubchenya, V.; Weber, C.; Äystö, J.

    2009-04-01

    A survey of neutron-deficient nuclides which can be produced via proton- and 3He -induced fusion-evaporation reactions in the A = 100 region was made using a Penning trap as a high-resolution mass filter. A comparison of the measured isotopic rates with a statistical model calculation for the proton-induced reactions shows the importance of using the precise binding energy values for the final reaction products. In particular, proton separation energies were found to play an important role in the evaporation process. In addition, accurate masses of 12 nuclides, 97-99, 101Pd , 100Ag , 101-105Cd and 102, 104In , were determined with uncertainties of less than 10keV.

  6. Cosmogenic nuclide age constraints on Middle Stone Age lithics from Niassa, Mozambique

    NASA Astrophysics Data System (ADS)

    Mercader, Julio; Gosse, John C.; Bennett, Tim; Hidy, Alan J.; Rood, Dylan H.

    2012-07-01

    The late phases of the Middle Stone Age (MSA) in the East African Rift System (EARS) are known for their evolutionary shifts and association with bottlenecks, transcontinental expansion, and climatic fluctuations. The chronology of MSA sites contemporaneous with these eco-demographic upheavals is uncertain because of the scarcity of datable sites and the poor understanding of their depositional and erosional histories. We apply terrestrial cosmogenic nuclide dating in a stratigraphic section with a complex exposure history to the study of the Luchamange Beds, a widespread sedimentological unit underlying MSA sites from the shores of Lake Niassa (Mozambican EARS). We use an innovative approach, which may be applicable elsewhere, to calculate their age using a Monte Carlo-based Bayesian model that links depth profiles of 26Al and 10Be, and uses other geomorphic and cosmogenic nuclide age constraints on episodic erosion and burial. The age of the basal Luchamange Beds is 42 + 77/-15 ka, and the MSA occupation on top is 29 + 3/-11 ka. These dates suggest temporal overlap between MSA and the earliest Later Stone Age and diversity in cultural manifestations at the end of the MSA.

  7. Carbon Isotope Composition of Ecosystem Respired Carbon Dioxide in Three Boreal Forest Ecosystems: Measurements and Model Calculations

    NASA Astrophysics Data System (ADS)

    Cai, T.; Flanagan, L. B.

    2007-12-01

    We conducted measurements of seasonal and inter-annual variation in the carbon isotope composition of ecosystem respired CO2 (δR) in aspen, black spruce and jack pine dominated ecosystems in northern Saskatchewan during 2004-2006 as part of the Fluxnet-Canada Research Network. All three sites showed relatively small variation (approximately -26 to -29 per mil) in δR values during the entire study. The measurements were strongly correlated with modeled δ13C values of ecosystem respired CO2. The model calculated leaf CO2 assimilation, stomatal conductance and chloroplast CO2 concentration separately for sunlit and shaded leaves within multiple canopy layers, and, therefore, allowed us to estimate canopy photosynthetic 13C discrimination. All three sites showed variation in canopy 13C discrimination in response to environmental conditions in a manner consistent with well-known leaf-level studies. Specifically, 13C discrimination was positively correlated with soil moisture and negatively correlated with photon flux density, air temperature and vapor pressure deficit. As a consequence a strong diurnal pattern was observed for 13C discrimination. The measured δR values also varied in response to environmental conditions in a manner consistent with well-known leaf-level studies of photosynthetic 13C discrimination, but with a dampened response caused by the contribution of heterotrophic respiration, which had a constant δ13C value. These results indicate that the stable isotope composition of respired CO2 is a useful ecosystem-scale tool to study constraints to photosynthesis and acclimation of ecosystems to environmental stress.

  8. Notre Dame Nuclear Database: A New Chart of Nuclides

    NASA Astrophysics Data System (ADS)

    Lee, Kevin; Khouw, Timothy; Fasano, Patrick; Mumpower, Matthew; Aprahamian, Ani

    2014-09-01

    Nuclear data is critical to research fields from medicine to astrophysics. We are creating a database, the Notre Dame Nuclear Database, which can store theoretical and experimental datasets. We place emphasis on storing metadata and user interaction with the database. Users are able to search in addition to the specific nuclear datum, the author(s), the facility where the measurements were made, the institution of the facility, and device or method/technique used. We also allow users to interact with the database by providing online search, an interactive nuclide chart, and a command line interface. The nuclide chart is a more descriptive version of the periodic table that can be used to visualize nuclear properties such as half-lives and mass. We achieve this by using D3 (Data Driven Documents), HTML, and CSS3 to plot the nuclides and color them accordingly. Search capabilities can be applied dynamically to the chart by using Python to communicate with MySQL, allowing for customization. Users can save the customized chart they create to any image format. These features provide a unique approach for researchers to interface with nuclear data. We report on the current progress of this project and will present a working demo that highlights each aspect of the aforementioned features. This is the first time that all available technologies are put to use to make nuclear data more accessible than ever before in a manner that is much easier and fully detailed. This is a first and we will make it available as open source ware.

  9. Facies composition calculated from the sonic, neutron, and density log suite, upper part of the Minnelusa Formation, Powder River basin, Wyoming

    USGS Publications Warehouse

    Schmoker, J.W.; Schenk, C.J.

    1988-01-01

    Sandstones and dolomites of the Permian upper part of the Minnelusa Formation are treated here as four-component systems consisting of fluid-filled pore space, quartz, dolomite, and anhydrite. Response equations of sonic, neutron, and density logs form a system of four simultaneous equations. With four equations and four unknowns, the composition of upper Minnelusa facies is defined by the three-log suite and can be calculated by solving a 4 ?? 4 matrix. Such calculations of facies composition help in establishing subsurface correlations and yield information on the diagenesis and physical character of upper Minnelusa sandstones and dolomites. Applications of composition calculations are illustrated by examples drawn from the area of the West Mellott field (T52N, R68W), where the upper Minnelusa is at depths of about 7000 ft (2100m). -from Authors

  10. ANDROS: A code for Assessment of Nuclide Doses and Risks with Option Selection

    SciTech Connect

    Begovich, C.L.; Sjoreen, A.L.; Ohr, S.Y.; Chester, R.O.

    1986-11-01

    ANDROS (Assessment of Nuclide Doses and Risks with Option Selection) is a computer code written to compute doses and health effects from atmospheric releases of radionuclides. ANDROS has been designed as an integral part of the CRRIS (Computerized Radiological Risk Investigation System). ANDROS reads air concentrations and environmental concentrations of radionuclides to produce tables of specified doses and health effects to selected organs via selected pathways (e.g., ingestion or air immersion). The calculation may be done for an individual at a specific location or for the population of the whole assessment grid. The user may request tables of specific effects for every assessment grid location. Along with the radionuclide concentrations, the code requires radionuclide decay data, dose and risk factors, and location-specific data, all of which are available within the CRRIS. This document is a user manual for ANDROS and presents the methodology used in this code.

  11. Steady-state creep of bent reinforced metal-composite plates with consideration of their reduced resistance to transverse shear 2. Analysis of calculated results

    NASA Astrophysics Data System (ADS)

    Yankovskii, A. P.

    2014-07-01

    Deformation of annular plates with different structures of helical reinforcement is studied. It is demonstrated that the use of the classical theory for calculating steady-state creep for thick reinforced plates subjected to bending leads to underprediction of the compliance of thin-walled metal-composite structures. It is also shown that there are significant shear strain rates in the binder of such plates, which has to be taken into account and which is mainly responsible for creep strain accumulation. Results calculated by two different models, which take into account the composite structure, are compared.

  12. ICoN, the Interactive Chart of Nuclides

    NASA Astrophysics Data System (ADS)

    Lee, Kevin; Mumpower, Matthew; Aprahamian, Ani

    2015-10-01

    Nuclear data is critical to research fields from medicine to astrophysics. The chart of nuclides is a more descriptive version of the periodic table that can be used to visualize nuclear properties such as half-lives and mass. We have created ICoN (simply short for Interactive Chart of Nuclides), an API which can be used to visualize theoretical and experimental datasets. This visualization is achieved by using D3 (Data Driven Documents), HTML, and CSS3 to plot the elements and color them accordingly. ICoN features many customization options that users can access that are dynamically applied to the chart without reloading the page. Users can save the customized chart they create to various formats. We have constructed these features in order to provide a unique approach for researchers to interface with nuclear data. ICoN can also be used on all electronic devices without loss of support. We report on the current progress of this project and will present a working demo that highlights each aspect of the aforementioned features. This is the first time that all available technologies are put to use to make nuclear data more accessible than ever before. This is a first and we will make it available as open source ware.

  13. Interpolations of nuclide-specific scattering kernels generated with Serpent

    SciTech Connect

    Scopatz, A.; Schneider, E.

    2012-07-01

    The neutron group-to-group scattering cross section is an essential input parameter for any multi-energy group physics model. However, if the analyst prefers to use Monte Carlo transport to generate group constants this data is difficult to obtain for a single species of a material. Here, the Monte Carlo code Serpent was modified to return the group transfer probabilities on a per-nuclide basis. This ability is demonstrated in conjunction with an essential physics reactor model where cross section perturbations are used to dynamically generate reactor state dependent group constants via interpolation from pre-computed libraries. The modified version of Serpent was therefore verified with three interpolation cases designed to test the resilience of the interpolation scheme to changes in intra-group fluxes. For most species, interpolation resulted in errors of less than 5% of transport-computed values. For important scatterers, such as {sup 1}H, errors less than 2% were observed. For nuclides with high errors ( > 10%), the scattering channel typically only had a small probability of occurring. (authors)

  14. Forbush decreases geomagnetic and atmospheric effects cosmogenic nuclides

    NASA Technical Reports Server (NTRS)

    Flueckiger, E. O.

    1986-01-01

    An overview and synthesis is given of recent developments that have occurred in the areas of Forbush decreases, geomagnetic and atmospheric effects, and cosmogenic nuclides. Experimental evidence has been found for substantial differences in the effects of the various types of interplanetary perturbations on cosmic rays, and for a dependence of these effects on the three-dimensional configuration of the interplanetary medium. In order to fully understand and to be able to simulate the solar cosmic ray particle access to the polar regions of the earth we need accurate models of the magnetospheric magnetic field. These models must include all major magnetospheric current systems (in particular the field aligned currents), and they should represent magnetically quiet time periods as well as different levels of geomagnetic activity. In the evolution of magnetospheric magnetic field models, cosmic ray and magnetospheric physicists should work closely together since cosmic ray measurements are a powerful additional tool in the study of the perturbed magnetosphere. In the field of cosmogenic nuclides, finally, exciting new results and developments follow in rapid succession. Thanks to new techniques and new isotopes the analysis of cosmic ray history has entered into a new dimension.

  15. Penning trap mass measurements of nuclides along the astrophysical rp- and νp- process paths

    NASA Astrophysics Data System (ADS)

    Clark, Jason

    2009-10-01

    X-ray bursters and supernovae are examples of explosive stellar phenomena in which nuclides are quickly produced in great quantities. Observed as x-ray bursts, thermonuclear runaways on the surface of neutron stars accreting material from its binary star companion create elements by a nucleosynthetic procoess which involves a series of rapid proton-capture reactions, termed the rp process. The timescale, nuclides produced, and energy released during the rp process are very sensitive to delays encountered at waiting-point nuclides, nuclides in which their slow β decay is more probable than net proton capture. A possible mechanism to bypass the waiting-point nuclides is through the νp process, in which (n,p) and (n,γ) reactions on the waiting-point nuclides, in addition to the proton-capture reactions, are possible. Supernovae are possible sites for the νp process as the proton-rich ejecta can absorb antineutrinos to produce the required free neutrons. It is this νp process which may resolve the long-standing discrepancy between the observed and predicted abundances of ^92Mo and ^94Mo. Proton-capture Q values of nuclides along the rp- and νp- process paths are required to accurately model the nucleosynthesis, especially at the waiting-point nuclides. In recent years, Penning traps have become the preferred tool to make precise mass measurements of stable and unstable nuclides. To make the best use of these devices in measuring the masses of radioactive nuclides, systems have been developed to quickly, cleanly, and efficiently transport the short-lived, weakly produced nuclides to the Penning traps. This talk will discuss the rp and νp nucleosynthetic processes and will highlight the precise Penning trap mass measurements of nuclides along these process paths.

  16. Bridging the timescales between thermochronological and cosmogenic nuclide data

    NASA Astrophysics Data System (ADS)

    Glotzbach, Christoph

    2015-04-01

    Reconstructing the evolution of Earth's landscape is a key to understand its future evolution and to identify the driving forces that shape Earth's surface. Cosmogenic nuclide and thermochronological methods are routinely used to quantify Earth surface processes over 102-104 yr and 106-107 yr, respectively (e.g. Lal 1991; Reiners and Ehlers 2005; von Blanckenburg 2006). A comparison of the rates of surface processes derived from these methods is, however, hampered by the large difference in their timescales. For instance, a constant erosion rate of 0.1 mm/yr yield an apatite (U-Th)/He age of ~24 Ma and a 10Be age of ~6 ka, respectively. Analytical methods that bridge this time gap are on the way, but are not yet fully established (e.g. Herman et al. 2010). A ready to use alternative are river profiles, which record the regional uplift history over 102-107 yr (e.g. Pritchard et al. 2009). Changes in uplift are retained in knickzones that propagate with a distinct velocity upstream, and therefore the time of an uplift event can be estimated. Here I present an integrative inverse modelling approach to simultaneously reconstruct river profiles, model thermochronological and cosmogenic nuclide data and to derive robust information about landscape evolution over thousands to millions of years. An efficient inversion routine is used to solve the forward problem and find the best uplift history and erosional parameters that reproduce the observed data. I test the performance of the algorithm by inverting a synthetic dataset and a dataset from the Sila massif (Italy). Results show that even complicated uplift histories can be reliably retrieved by the combined interpretation of river profiles, thermochronological and cosmogenic nuclide data. References Gallagher, K., Brown, R. & Johnson, C. (1998): Fission track analysis and its applications to geological problems. - Annu. Rev. Earth Planet., 26: 519-572. Herman, F., Rhodes, E.J., Braun, J. & Heiniger, L. (2010): Uniform

  17. Nuclides.net: A Web-Based Environment for Nuclear Data and Applications

    SciTech Connect

    Galy, J.; Magill, J.

    2005-05-24

    An interactive multimedia tool, Nuclides.net, has been developed at the Institute for Transuranium Elements. The Nuclides.net 'integrated environment' is a suite of computer programs ranging from a powerful user-friendly interface, which allows the user to navigate the nuclides chart and explore the properties of nuclides, to various computational modules. Through this powerful interface, the user can access a wide variety of nuclear data including, e.g., radioactive decay data, cross sections, fission yields, etc. from international recognized sources.

  18. ACDOS1: a computer code to calculate dose rates from neutron activation of neutral beamlines and other fusion-reactor components

    SciTech Connect

    Keney, G.S.

    1981-08-01

    A computer code has been written to calculate neutron induced activation of neutral-beam injector components and the corresponding dose rates as a function of geometry, component composition, and time after shutdown. The code, ACDOS1, was written in FORTRAN IV to calculate both activity and dose rates for up to 30 target nuclides and 50 neutron groups. Sufficient versatility has also been incorporated into the code to make it applicable to a variety of general activation problems due to neutrons of energy less than 20 MeV.

  19. Removal of radio nuclides of the U- and Th- series from aqueous solutions by adsorption onto Polyacryamide-expanded perlite: Effects of pH, concentration and temperature

    NASA Astrophysics Data System (ADS)

    Akkaya, Recep

    2012-10-01

    Poly (Acryamide-expanded perlite) [P(AAm-EP)], was synthesized. The influence of process parameters: initial pH and five radio nuclides of the U- and Th- series (TI+, Ra2+, Bi3+, Ac3+ and Pb2+ in a leaching solution) concentration, on sorption thermodynamic was studied and discussed. The five natural radio nuclides were counted by gamma spectrometer using a type NAI (Tl) detector. The amounts of five radio nuclides sorbed at equlibrium were well represented by Langmuir and Freundlich type isotherms. The Langmuir adsorption capacities (XL) were in the order of 208Tl (0.4 MBq kg-1)>212Pb and 212Bi (0.3 MBq kg-1)>228Ac and (0.1 MBq kg-1)>226Ra (0.04 MBq kg-1). These results demonstrated that P(AAm-EP) had high affinity to the five natural radio nuclides. In order to specify the type of adsorption reaction, thermodynamic parameters such as the standard enthalpy, entropy, and Gibbs free energy were also determined. It was also demonstrated that the adsorption mechanism was spontaneous (ΔG<0), the process was exothermic (ΔH<0) thus increasing entropy (ΔS>0). The composite was reused for four more times after regeneration without any detectable changes either in its structure or adsorptive capability.

  20. Multi-nuclide AMS system at the University of Tsukuba

    SciTech Connect

    Sasa, Kimikazu; Takahashi, Tsutomu

    2010-05-12

    A multi-nuclide AMS system on the 12UD Pelletron tandem accelerator at the University of Tsukuba (Tsukuba AMS system) can measure environmental levels of long-lived radioisotopes of {sup 14}C, {sup 26}Al, {sup 36}Cl and {sup 129}I by employing a molecular pilot beam. AMS is an ultrasensitive technique for the study of long-lived radioisotopes, and stable isotopes at very low abundances. The high terminal voltage has an advantage in the detection of heavy radioisotopes. Much progress has been made in the development of new AMS techniques. For example, a standard deviation of the fluctuation for the {sup 36}Cl/Cl ratio is +- 2%, and the effective detection limit is better than 1x10{sup -15}. In recent years, the main research field of the 12UD Pelletron tandem accelerator has shifted to accelerator mass spectrometry (AMS) research from nuclear physics. This report presents an overview of the Tsukuba AMS system.

  1. A MATLAB toolbox and Excel workbook for calculating the densities, seismic wave speeds, and major element composition of minerals and rocks at pressure and temperature

    NASA Astrophysics Data System (ADS)

    Abers, Geoffrey A.; Hacker, Bradley R.

    2016-02-01

    To interpret seismic images, rock seismic velocities need to be calculated at elevated pressure and temperature for arbitrary compositions. This technical report describes an algorithm, software, and data to make such calculations from the physical properties of minerals. It updates a previous compilation and Excel® spreadsheet and includes new MATLAB® tools for the calculations. The database of 60 mineral end-members includes all parameters needed to estimate density and elastic moduli for many crustal and mantle rocks at conditions relevant to the upper few hundreds of kilometers of Earth. The behavior of α and β quartz is treated as a special case, owing to its unusual Poisson's ratio and thermal expansion that vary rapidly near the α-β transition. The MATLAB tools allow integration of these calculations into a variety of modeling and data analysis projects.

  2. Fission barriers at the end of the chart of the nuclides

    SciTech Connect

    Möller, Peter; Sierk, Arnold J.; Ichikawa, Takatoshi; Iwamoto, Akira; Mumpower, Matthew

    2015-02-12

    We present calculated fission-barrier heights for 5239 nuclides for all nuclei between the proton and neutron drip lines with 171 ≤ A ≤ 330. The barriers are calculated in the macroscopic-microscopic finite-range liquid-drop (FRLDM) with a 2002 set of macroscopic-model parameters. The saddle-point energies are determined from potential-energy surfaces based on more than five million different shapes, defined by five deformation parameters in the three-quadratic-surface shape parametrization: elongation, neck diameter, left-fragment spheroidal deformation, right-fragment spheroidal deformation, and nascent-fragment mass asymmetry. The energy of the ground state is determined by calculating the lowest-energy configuration in both the Nilsson perturbed-spheroid (ϵ) and the spherical-harmonic (β) parametrizations, including axially asymmetric deformations. The lower of the two results (correcting for zero-point motion) is defined as the ground-state energy. The effect of axial asymmetry on the inner barrier peak is calculated in the (ϵ,γ) parametrization. We have earlier benchmarked our calculated barrier heights to experimentally extracted barrier parameters and found average agreement to about one MeV for known data across the nuclear chart. Here we do additional benchmarks and investigate the qualitative and, when possible, quantitative agreement and/or consistency with data on β-delayed fission, isotope generation along prompt-neutron-capture chains in nuclear-weapons tests, and superheavy-element stability. In addition these studies all indicate that the model is realistic at considerable distances in Z and N from the region of nuclei where its parameters were determined.

  3. Fission barriers at the end of the chart of the nuclides

    DOE PAGESBeta

    Möller, Peter; Sierk, Arnold J.; Ichikawa, Takatoshi; Iwamoto, Akira; Mumpower, Matthew

    2015-02-12

    We present calculated fission-barrier heights for 5239 nuclides for all nuclei between the proton and neutron drip lines with 171 ≤ A ≤ 330. The barriers are calculated in the macroscopic-microscopic finite-range liquid-drop (FRLDM) with a 2002 set of macroscopic-model parameters. The saddle-point energies are determined from potential-energy surfaces based on more than five million different shapes, defined by five deformation parameters in the three-quadratic-surface shape parametrization: elongation, neck diameter, left-fragment spheroidal deformation, right-fragment spheroidal deformation, and nascent-fragment mass asymmetry. The energy of the ground state is determined by calculating the lowest-energy configuration in both the Nilsson perturbed-spheroid (ϵ) andmore » the spherical-harmonic (β) parametrizations, including axially asymmetric deformations. The lower of the two results (correcting for zero-point motion) is defined as the ground-state energy. The effect of axial asymmetry on the inner barrier peak is calculated in the (ϵ,γ) parametrization. We have earlier benchmarked our calculated barrier heights to experimentally extracted barrier parameters and found average agreement to about one MeV for known data across the nuclear chart. Here we do additional benchmarks and investigate the qualitative and, when possible, quantitative agreement and/or consistency with data on β-delayed fission, isotope generation along prompt-neutron-capture chains in nuclear-weapons tests, and superheavy-element stability. In addition these studies all indicate that the model is realistic at considerable distances in Z and N from the region of nuclei where its parameters were determined.« less

  4. Fission barriers at the end of the chart of the nuclides

    NASA Astrophysics Data System (ADS)

    Möller, Peter; Sierk, Arnold J.; Ichikawa, Takatoshi; Iwamoto, Akira; Mumpower, Matthew

    2015-02-01

    We present calculated fission-barrier heights for 5239 nuclides for all nuclei between the proton and neutron drip lines with 171 ≤A ≤330 . The barriers are calculated in the macroscopic-microscopic finite-range liquid-drop model with a 2002 set of macroscopic-model parameters. The saddle-point energies are determined from potential-energy surfaces based on more than 5 000 000 different shapes, defined by five deformation parameters in the three-quadratic-surface shape parametrization: elongation, neck diameter, left-fragment spheroidal deformation, right-fragment spheroidal deformation, and nascent-fragment mass asymmetry. The energy of the ground state is determined by calculating the lowest-energy configuration in both the Nilsson perturbed-spheroid (ɛ ) and the spherical-harmonic (β ) parametrizations, including axially asymmetric deformations. The lower of the two results (correcting for zero-point motion) is defined as the ground-state energy. The effect of axial asymmetry on the inner barrier peak is calculated in the (ɛ ,γ ) parametrization. We have earlier benchmarked our calculated barrier heights to experimentally extracted barrier parameters and found average agreement to about 1 MeV for known data across the nuclear chart. Here we do additional benchmarks and investigate the qualitative and, when possible, quantitative agreement and/or consistency with data on β -delayed fission, isotope generation along prompt-neutron-capture chains in nuclear-weapons tests, and superheavy-element stability. These studies all indicate that the model is realistic at considerable distances in Z and N from the region of nuclei where its parameters were determined.

  5. Calculation of the Rate of Combustion of a Metallized Composite Solid Propellant with Allowance for the Size Distribution of Agglomerates

    NASA Astrophysics Data System (ADS)

    Poryazov, V. A.; Krainov, A. Yu.

    2016-06-01

    A physicomathematical model of combustion of a metallized composite solid propellant based on ammonium perchlorate has been presented. The model takes account of the thermal effect of decomposition of a condensed phase (c phase), convection, diffusion, the exothermal chemical reaction in a gas phase, the heating and combustion of aluminum particles in the gas flow, and the velocity lag of the particles behind the gas. The influence of the granulometric composition of aluminum particles escaping from the combustion surface on the linear rate of combustion has been investigated. It has been shown that information not only on the kinetics of chemical reactions in the gas phase, but also on the granulometric composition of aluminum particles escaping from the surface of the c phase into the gas, is of importance for determination of the linear rate of combustion.

  6. Calculation of the Rate of Combustion of a Metallized Composite Solid Propellant with Allowance for the Size Distribution of Agglomerates

    NASA Astrophysics Data System (ADS)

    Poryazov, V. A.; Krainov, A. Yu.

    2016-05-01

    A physicomathematical model of combustion of a metallized composite solid propellant based on ammonium perchlorate has been presented. The model takes account of the thermal effect of decomposition of a condensed phase (c phase), convection, diffusion, the exothermal chemical reaction in a gas phase, the heating and combustion of aluminum particles in the gas flow, and the velocity lag of the particles behind the gas. The influence of the granulometric composition of aluminum particles escaping from the combustion surface on the linear rate of combustion has been investigated. It has been shown that information not only on the kinetics of chemical reactions in the gas phase, but also on the granulometric composition of aluminum particles escaping from the surface of the c phase into the gas, is of importance for determination of the linear rate of combustion.

  7. Composition.

    ERIC Educational Resources Information Center

    Nemanich, Donald, Ed.

    1974-01-01

    The articles in this special issue of the "Illinois English Bulletin" concern the state of composition instruction at the secondary and college levels. The titles and authors are "Monologues or Dialogues? A Plea for Literacy" by Dr. Alfred J. Lindsey, "Teaching Composition: Curiouser and Curiouser" by Denny Brandon, and "Teaching Writing to High…

  8. Excited states in the proton-unbound nuclide 158Ta

    NASA Astrophysics Data System (ADS)

    Carroll, R. J.; Page, R. D.; Joss, D. T.; O'Donnell, D.; Uusitalo, J.; Darby, I. G.; Andgren, K.; Auranen, K.; Bönig, S.; Cederwall, B.; Doncel, M.; Drummond, M. C.; Eeckhaudt, S.; Grahn, T.; Gray-Jones, C.; Greenlees, P. T.; Hadinia, B.; HerzáÅ, A.; Jakobsson, U.; Jones, P. M.; Julin, R.; Juutinen, S.; Konki, J.; Kröll, T.; Leino, M.; Leppänen, A.-P.; McPeake, C.; Nyman, M.; Pakarinen, J.; Partanen, J.; Peura, P.; Rahkila, P.; Revill, J.; Ruotsalainen, P.; Sandzelius, M.; Sarén, J.; Sayǧi, B.; Scholey, C.; Seweryniak, D.; Simpson, J.; Sorri, J.; Stolze, S.; Taylor, M. J.; Thornthwaite, A.

    2016-03-01

    Excited states in the neutron-deficient odd-odd proton-unbound nuclide 158Ta have been investigated in two separate experiments. In the first experiment, 166Ir nuclei were produced in the reactions of 380 MeV 78Kr ions with an isotopically enriched 92Mo target. The α -decay chain of the 9+ state in 166Ir was analyzed. Fine structure in the α decay of the 9+ state in 162Re established a 66 keV difference in excitation energy between the lowest-lying 9+ and 10+ states in 158Ta. Higher-lying states in 158Ta were populated in the reactions of 255 MeV 58Ni ions with an isotopically enriched 102Pd target. Gamma-ray decay paths that populate, depopulate, and bypass a 19- isomeric state have been identified. The general features of the deduced level scheme are discussed and the prospects for observing proton emission branches from excited states are considered.

  9. Modified microspheres for cleaning liquid wastes from radioactive nuclides

    SciTech Connect

    Danilin, Lev; Drozhzhin, Valery

    2007-07-01

    An effective solution of nuclear industry problems related to deactivation of technological and natural waters polluted with toxic and radioactive elements is the development of inorganic sorbents capable of not only withdrawing radioactive nuclides, but also of providing their subsequent conservation under conditions of long-term storage. A successful technical approach to creation of sorbents can be the use of hollow aluminosilicate microspheres. Such microspheres are formed from mineral additives during coal burning in furnaces of boiler units of electric power stations. Despite some reduction in exchange capacity per a mass unit of sorbents the latter have high kinetic characteristics that makes it possible to carry out the sorption process both in static and dynamic modes. Taking into account large industrial resources of microspheres as by-products of electric power stations, a comparative simplicity of the modification process, as well as good kinetic and capacitor characteristics, this class of sorbents can be considered promising enough for solving the problems of cleaning liquid radioactive wastes of various pollution levels. (authors)

  10. Engineering refinements to overcome default nuclide regulatory constraints

    NASA Astrophysics Data System (ADS)

    Finn, R.; Capitelli, P.; Sheh, Y.; Lom, C.; Graham, M.; Germain, J. St.

    2005-12-01

    The "classical" positron emitting radionuclides include oxygen-15, nitrogen-13 and carbon-11 which possess unique properties for medical imaging. They are radionuclides of the fundamental elements of biological matter. They each possess short half-lives which allow their use in designed radiotracers for clinical investigations with minimal risk and they are readily able to be produced in sufficient activities by low energy nuclear reactions. At present several accelerator manufacturers offer production packages for these radionuclides emphasizing targetry with consideration of the cyclotron extracted energies for nuclide production and on-line chemistry systems for the continuous production of specific precursors or radiotracers. Following the installation and acceptance of the MSKCC TR 19/9 Cyclotron, our experience with the procured chemistry module for the preparation of oxygen-15 labeled water has forced us to examine the design and the operation of the synthetic unit with a view toward the state of New York's regulations addressing the environmental pollution from radioactive materials. The chemistry module was refined with subtle modifications to the chemistry procedure/unit and our experience with the unit is presented as an example of our approach to insure regulatory compliance.

  11. Implementation of Improved Transverse Shear Calculations and Higher Order Laminate Theory Into Strain Rate Dependent Analyses of Polymer Matrix Composites

    NASA Technical Reports Server (NTRS)

    Zhu, Lin-Fa; Kim, Soo; Chattopadhyay, Aditi; Goldberg, Robert K.

    2004-01-01

    A numerical procedure has been developed to investigate the nonlinear and strain rate dependent deformation response of polymer matrix composite laminated plates under high strain rate impact loadings. A recently developed strength of materials based micromechanics model, incorporating a set of nonlinear, strain rate dependent constitutive equations for the polymer matrix, is extended to account for the transverse shear effects during impact. Four different assumptions of transverse shear deformation are investigated in order to improve the developed strain rate dependent micromechanics model. The validities of these assumptions are investigated using numerical and theoretical approaches. A method to determine through the thickness strain and transverse Poisson's ratio of the composite is developed. The revised micromechanics model is then implemented into a higher order laminated plate theory which is modified to include the effects of inelastic strains. Parametric studies are conducted to investigate the mechanical response of composite plates under high strain rate loadings. Results show the transverse shear stresses cannot be neglected in the impact problem. A significant level of strain rate dependency and material nonlinearity is found in the deformation response of representative composite specimens.

  12. The concentration of short-lived spontaneously fissioning nuclides from iron-manganes nodules

    NASA Astrophysics Data System (ADS)

    Maslov, O. D.

    2016-03-01

    The paper reports on the observation of the spontaneously fissioning nuclides as a result of hydrochemical and high-temperature processing of iron-manganese nodules. The spontaneous fission in the samples obtained was measured by the track method using electrochemical etching, and nuclides with T 1/2 = 15 d, T 1/2 = 25 d that is similar in chemical properties to Os and T 1/2 = 62 d, (similar in chemical properties to Pb and Ra) were detected. The content of the parent nuclide in iron-manganese nodules corresponds to 4 × 10-14-8 × 10-14 g/g.

  13. The Navy/NASA Engine Program (NNEP89): Interfacing the program for the calculation of complex Chemical Equilibrium Compositions (CEC)

    NASA Technical Reports Server (NTRS)

    Gordon, Sanford

    1991-01-01

    The NNEP is a general computer program for calculating aircraft engine performance. NNEP has been used extensively to calculate the design and off-design (matched) performance of a broad range of turbine engines, ranging from subsonic turboprops to variable cycle engines for supersonic transports. Recently, however, there has been increased interest in applications for which NNEP is not capable of simulating, such as the use of alternate fuels including cryogenic fuels and the inclusion of chemical dissociation effects at high temperatures. To overcome these limitations, NNEP was extended by including a general chemical equilibrium method. This permits consideration of any propellant system and the calculation of performance with dissociation effects. The new extended program is referred to as NNEP89.

  14. New effective moduli of isotropic viscoelastic composites. Part II. Comparison of approximate calculation with the analytical solution

    NASA Astrophysics Data System (ADS)

    Kupriyanov, N. A.; Simankin, F. A.; Manabaev, K. K.

    2016-04-01

    A new approximate algorithm for calculating a stress-strain state of viscoelastic bodies is used. The algorithm is based on the derivation of the expressions of time-effective modules. These modules are obtained by iterative changes, compressing the fork of Voigt-Reuss. As an example the analytic solution about the action of a concentrated force on the viscoelastic half-space is compared with the approximate solution. Numerical calculations are performed for a wide range of relaxation characteristics of a viscoelastic half-space. Results of the comparison of stresses and displacements with the analytic solution give coincidence within 3... 15%.

  15. Assessment of experimental bond dissociation energies using composite ab initio methods and evaluation of the performances of density functional methods in the calculation of bond dissociation energies.

    PubMed

    Feng, Yong; Liu, Lei; Wang, Jin-Ti; Huang, Hao; Guo, Qing-Xiang

    2003-01-01

    Composite ab initio CBS-Q and G3 methods were used to calculate the bond dissociation energies (BDEs) of over 200 compounds listed in CRC Handbook of Chemistry and Physics (2002 ed.). It was found that these two methods agree with each other excellently in the calculation of BDEs, and they can predict BDEs within 10 kJ/mol of the experimental values. Using these two methods, it was found that among the examined compounds 161 experimental BDEs are valid because the standard deviation between the experimental and theoretical values for them is only 8.6 kJ/mol. Nevertheless, 40 BDEs listed in the Handbook may be highly inaccurate as the experimental and theoretical values for them differ by over 20 kJ/mol. Furthermore, 11 BDEs listed in the Handbook may be seriously flawed as the experimental and theoretical values for them differ by over 40 kJ/mol. Using the 161 cautiously validated experimental BDEs, we then assessed the performances of the standard density functional (DFT) methods including B3LYP, B3P86, B3PW91, and BH&HLYP in the calculation of BDEs. It was found that the BH&HLYP method performed poorly for the BDE calculations. B3LYP, B3P86, and B3PW91, however, performed reasonably well for the calculation of BDEs with standard deviations of about 12.1-18.0 kJ/mol. Nonetheless, all the DFT methods underestimated the BDEs by 4-17 kJ/mol in average. Sometimes, the underestimation by the DFT methods could be as high as 40-60 kJ/mol. Therefore, the DFT methods were more reliable for relative BDE calculations than for absolute BDE calculations. Finally, it was observed that the basis set effects on the BDEs calculated by the DFT methods were usually small except for the heteroatom-hydrogen BDEs. PMID:14632451

  16. A new tool for the search of nuclides with properties suitable for nuclear solid state physics based on the Evaluated Nuclear Structure Data Files

    NASA Astrophysics Data System (ADS)

    Nagl, M. A.; Barbosa, M. B.; Vetter, U.; Correia, J. G.; Hofsäss, H. C.

    2013-10-01

    A software tool for the displaying of nuclear decay schemes, the calculation of angular γ emission anisotropies, and the automated search for appropriate decay cascade properties based on the Evaluated Nuclear Structure Data Files (ENSDF) was created and published for free download. After a short introduction of this tool, candidate nuclides for time differential perturbed γ-γ angular correlation (TDPAC) measurements are presented. These candidates are grouped according to their parent nuclides’ half-life periods in groups for online, on-site, and off-site measurements. For all candidates angular correlation coefficients (also called anisotropy values) were computed and are shown alongside magnetic and quadrupole moments from the ENSDF database and other sources. An extension of the presented software for the search of nuclides for Mössbauer spectroscopy, Nuclear Resonant Scattering, and other methods is easily possible.

  17. Phase II Nuclide Partition Laboratory Study Influence of Cellulose Degradation Products on the Transport of Nuclides from SRS Shallow Land Burial Facilities

    SciTech Connect

    Serkiz, S.M.

    1999-10-04

    Degradation products of cellulosic materials (e.g., paper and wood products) can significantly influence the subsurface transport of metals and radionuclides. Codisposal of radionuclides with cellulosic materials in the E-Area slit trenches at the Savannah River Site (SRS) is, therefore, expected to influence nuclide fate and transport in the subsurface. Due to the complexities of these systems and the scarcity of site-specific data, the effects of cellulose waste loading and its subsequent influence on nuclide transport are not well established.

  18. Recommended Partition Coefficient (Kd) Values for Nuclide Partitioning in the Presence of Cellulose Degradation Products

    SciTech Connect

    Serkiz, S.M.

    2001-02-23

    This report documents the data analysis of the results of the described laboratory studies in order to recommend Kd values for use in Performance Assessment modeling of nuclide transport in the presence of CDP.

  19. (1) Selective separation and solidification of radioactive nuclides by zeolites

    NASA Astrophysics Data System (ADS)

    Mimura, Hitoshi; Sato, Nobuaki; Kirishima, Akira

    Massive tsunami generated by the Great East Japan Earthquake attacked the Fukushima Daiichi Nuclear Power Plant and caused the nuclear accident of level 7 to overturn the safety myth of the nuclear power generation. The domestic worst accident does not yet reach the convergence, and many inhabitants around the power plant are forced to double pains of earthquake disaster and nuclear accident. Large amounts of high-activity-level water over 200,000 tons are accumulated on the basement floor of each turbine building, which is a serious obstacle to take measures for the nuclear accident. For the decontamination of high-activity-level water containing seawater, the inorganic ion-exchangers having high selectivity are effective especially for the selective removal of radioactive Cs. On the other hand, radioactive Cs and I released into the atmosphere from the power plant spread widely around Fukushima prefecture, and the decontamination of rainwater and soil become the urgent problem. At present, passing about four months after nuclear accident, the radioactive nuclides of 137Cs and 134Cs are mainly contained in the high-activity-level water and the selective adsorbents for radioactive Cs play an important part in the decontamination. Since the construction of original decontamination system is an urgent necessity, selective separation methods using inorganic ion-exchangers are greatly expected. From the viewpoint of cost efficiency and high Cs-selectivity, natural zeolites are effective for the decontamination of radioactive Cs. This special issue deals with the selective separation and solidification of radioactive Cs and Sr using zeolites.

  20. Composites

    SciTech Connect

    Chou, T.; McCullough, R.L.; Pipes, R.B.

    1986-10-01

    The degree of control over material properties that is typified by hybrid composites is transforming engineering design. In part because homogeneous materials such as metals and alloys do not offer comparable control, specifying a material and designing a component have traditionally taken place separately. As composites begin to replace traditional materials in fields and such as aerospace, component design and the specification of a material are merging and becoming aspects of a single process. The controllable microstructure of a composite allows it to be tailored to match the distribution of stresses to which it will be subject. At the same time components must come to reflect the distinctive nature of composites: their directional properties and the intricate forms they can be given through processes such as injection molding, filament winding and three-dimensional weaving. The complexity inherent in conceiving components and their materials at the same time suggests engineering design will grow increasingly dependent on computers and multidisciplinary teams. Such an approach will harness the full potential of composites for the technologies of the future. 10 figures.

  1. Measurements of Cosmogenic Nuclides in and their Significance for Samples Returned from Asteroids

    NASA Technical Reports Server (NTRS)

    Nishiizumi, K.; Herzog, G. F.; Reedy, R. C.

    2000-01-01

    Nuclear interactions of cosmic rays with matter produce cosmogenic nuclides (CNs). Ever since they were first measured nearly 50 years ago, cosmogenic nuclides have been used to infer the irradiation histories of terrestrial and extraterrestrial materials. Here we call for an extension of such measurements to samples returned from an asteroidal surface. The information gained in this way will be important for elucidating the evolution of the asteroidal surface. Additional information is contained in the original extended abstract.

  2. Investigation of Naturally Occurring Radio Nuclides in Shir-kuh Granites

    SciTech Connect

    Mazarei, Mohammad Mehdi; Zarei, Mojtaba

    2011-12-26

    One of the principle natural radiation resources is Granite which can be dangerous for human because of its radiations. Based on this fact, in this research we attempt to specify the activity amount of these natural radio nuclides, existing in Shir-kuh Granite of Yazd state. To specify the activity amount of this natural radio nuclides, it has been applied the measurement method of Gamma spectroscopy using high purity Germanium (HPGe) detector.

  3. Investigation of Naturally Occurring Radio Nuclides in Shir-kuh Granites

    NASA Astrophysics Data System (ADS)

    Mazarei, Mohammad Mehdi; Zarei, Mojtaba

    2011-12-01

    One of the principle natural radiation resources is Granite which can be dangerous for human because of its radiations. Based on this fact, in this research we attempt to specify the activity amount of these natural radio nuclides, existing in Shir-kuh Granite of Yazd state. To specify the activity amount of this natural radio nuclides, it has been applied the measurement method of Gamma spectroscopy using high purity Germanium (HPGe) detector.

  4. MAGMIX: a basic program to calculate viscosities of interacting magmas of differing composition, temperature, and water content

    USGS Publications Warehouse

    Frost, T.P.; Lindsay, J.R.

    1988-01-01

    MAGMIX is a BASIC program designed to predict viscosities at thermal equilibrium of interacting magmas of differing compositions, initial temperatures, crystallinities, crystal sizes, and water content for any mixing proportion between end members. From the viscosities of the end members at thermal equilibrium, it is possible to predict the styles of magma interaction expected for different initial conditions. The program is designed for modeling the type of magma interaction between hypersthenenormative magmas at upper crustal conditions. Utilization of the program to model magma interaction at pressures higher than 200 MPa would require modification of the program to account for the effects of pressure on heat of fusion and magma density. ?? 1988.

  5. Calculation of water equivalent thickness of materials of arbitrary density, elemental composition and thickness in proton beam irradiation.

    PubMed

    Zhang, Rui; Newhauser, Wayne D

    2009-03-21

    In proton therapy, the radiological thickness of a material is commonly expressed in terms of water equivalent thickness (WET) or water equivalent ratio (WER). However, the WET calculations required either iterative numerical methods or approximate methods of unknown accuracy. The objective of this study was to develop a simple deterministic formula to calculate WET values with an accuracy of 1 mm for materials commonly used in proton radiation therapy. Several alternative formulas were derived in which the energy loss was calculated based on the Bragg-Kleeman rule (BK), the Bethe-Bloch equation (BB) or an empirical version of the Bethe-Bloch equation (EBB). Alternative approaches were developed for targets that were 'radiologically thin' or 'thick'. The accuracy of these methods was assessed by comparison to values from an iterative numerical method that utilized evaluated stopping power tables. In addition, we also tested the approximate formula given in the International Atomic Energy Agency's dosimetry code of practice (Technical Report Series No 398, 2000, IAEA, Vienna) and stopping power ratio approximation. The results of these comparisons revealed that most methods were accurate for cases involving thin or low-Z targets. However, only the thick-target formulas provided accurate WET values for targets that were radiologically thick and contained high-Z material. PMID:19218739

  6. Calculation of water equivalent thickness of materials of arbitrary density, elemental composition and thickness in proton beam irradiation

    PubMed Central

    Zhang, Rui; Newhauser, Wayne D

    2014-01-01

    In proton therapy, the radiological thickness of a material is commonly expressed in terms of water equivalent thickness (WET) or water equivalent ratio (WER). However, the WET calculations required either iterative numerical methods or approximate methods of unknown accuracy. The objective of this study was to develop a simple deterministic formula to calculate WET values with an accuracy of 1 mm for materials commonly used in proton radiation therapy. Several alternative formulas were derived in which the energy loss was calculated based on the Bragg–Kleeman rule (BK), the Bethe–Bloch equation (BB) or an empirical version of the Bethe–Bloch equation (EBB). Alternative approaches were developed for targets that were ‘radiologically thin’ or ‘thick’. The accuracy of these methods was assessed by comparison to values from an iterative numerical method that utilized evaluated stopping power tables. In addition, we also tested the approximate formula given in the International Atomic Energy Agency's dosimetry code of practice (Technical Report Series No 398, 2000, IAEA, Vienna) and stopping power ratio approximation. The results of these comparisons revealed that most methods were accurate for cases involving thin or low-Z targets. However, only the thick-target formulas provided accurate WET values for targets that were radiologically thick and contained high-Z material. PMID:19218739

  7. Calculation of water equivalent thickness of materials of arbitrary density, elemental composition and thickness in proton beam irradiation

    NASA Astrophysics Data System (ADS)

    Zhang, Rui; Newhauser, Wayne D.

    2009-03-01

    In proton therapy, the radiological thickness of a material is commonly expressed in terms of water equivalent thickness (WET) or water equivalent ratio (WER). However, the WET calculations required either iterative numerical methods or approximate methods of unknown accuracy. The objective of this study was to develop a simple deterministic formula to calculate WET values with an accuracy of 1 mm for materials commonly used in proton radiation therapy. Several alternative formulas were derived in which the energy loss was calculated based on the Bragg-Kleeman rule (BK), the Bethe-Bloch equation (BB) or an empirical version of the Bethe-Bloch equation (EBB). Alternative approaches were developed for targets that were 'radiologically thin' or 'thick'. The accuracy of these methods was assessed by comparison to values from an iterative numerical method that utilized evaluated stopping power tables. In addition, we also tested the approximate formula given in the International Atomic Energy Agency's dosimetry code of practice (Technical Report Series No 398, 2000, IAEA, Vienna) and stopping power ratio approximation. The results of these comparisons revealed that most methods were accurate for cases involving thin or low-Z targets. However, only the thick-target formulas provided accurate WET values for targets that were radiologically thick and contained high-Z material.

  8. 10Be concentrations and the long-term fate of particle-reactive nuclides in five soil profiles from California

    NASA Astrophysics Data System (ADS)

    Monaghan, M. C.; Krishnaswami, S.; Thomas, J. H.

    1983-10-01

    Concentration-depth profiles of cosmic-ray-produced 10Be ( t1/2 = 1.5m.y.) have been measured by accelerator-mass spectrometry in five soil profiles. These measurements were made in an effort (1) to understand the retentivity of soil surfaces for particle-reactive tracers depositing from the atmosphere on time scales of 10 4-10 6 years, and (2) to explore the application of 10Be as a chronometer of geomorphic surface age. The profiles sampled are from two wave-cut terraces located near Mendocino, California, a table mountain top and an alluvial fan, both located near Friant, California. The ages of the Mendocino terraces are inferred to be (1-5) × 10 5 years based on amino-stratigraphic correlations and models of terrace evolution; those of the table mountain top and alluvial fan are 9.5 × 10 6 years and 6.0 × 10 5 years, respectively, based on K-Ar analyses. All the surfaces sampled are nearly flat and exhibit few erosional features. In addition to 10Be we measured 210Pb, 239,240Pu and 7Be to ascertain the retentivity of the soils for particle-reactive nuclides and to assess the present-day delivery rate of nuclides from the atmosphere. The 7Be inventory is 4.0 dpm/cm 2 similar to those observed at nearby locations. The inventories of 210Pb and Pu isotopes conform to those predicted from model calculations and suggest that the soil surfaces sampled retain the entire burden of particle-reactive nuclides delivered to them over short time scales, ˜ 100 years. The 10Be concentrations in the sample range between (0.2 and 7) × 10 8 atoms/g soil and show strong correlations with leachable Fe and/or Al. The inventory of 10Be in the soil domain sampled is 1-2 orders of magnitude lower than that expected from the geological age of the surface and an average delivery rate of 10Be from the atmosphere, 5.2 × 10 5 atoms/cm 2 yr. The low inventory of 10Be is attributed to its loss from the soil domain sampled by solution transport. Based on a simple ☐-model type

  9. Computer Program for Calculation of Complex Chemical Equilibrium Compositions, Rocket Performance, Incident and Reflected Shocks, and Chapman-Jouguet Detonations. Interim Revision, March 1976

    NASA Technical Reports Server (NTRS)

    Gordon, S.; Mcbride, B. J.

    1976-01-01

    A detailed description of the equations and computer program for computations involving chemical equilibria in complex systems is given. A free-energy minimization technique is used. The program permits calculations such as (1) chemical equilibrium for assigned thermodynamic states (T,P), (H,P), (S,P), (T,V), (U,V), or (S,V), (2) theoretical rocket performance for both equilibrium and frozen compositions during expansion, (3) incident and reflected shock properties, and (4) Chapman-Jouguet detonation properties. The program considers condensed species as well as gaseous species.

  10. Modeling of nuclide release from low-level radioactive paraffin waste: a comparison of simulated and real waste.

    PubMed

    Kim, Ju Youl; Kim, Chang Lak; Chung, Chang Hyun

    2002-10-01

    Nuclide leaching models based on mass transfer theory are reviewed and evaluated to analyze the leaching test results of simulated and real paraffin waste from Korean nuclear power plants (NPPs). An empirical model (EM), bulk diffusion model (BDM), coupled diffusion/dissolution model (CDDM), shrinking core model (SCM), modified SCM (MSCM), and uniform reaction model (URM) are selected for comparison. In case of simulated paraffin waste form, the experimental results are satisfactorily explained by the SCM which is based on a diffusion-controlled dissolution reaction. Leaching behavior of real paraffin waste form is well predicted by URM that considers inter-aggregated porous medium and intra-aggregated porous medium separately. If real paraffin waste forms are manufactured with relatively uniform composition, their leaching behaviors are expected to be similar to those of simulated paraffin waste forms. PMID:12169419

  11. A new methodology to calculate the environmental protection index (Ep). A case study applied to a company producing composite materials.

    PubMed

    Siracusa, G; La Rosa, A D; Sterlini, S E

    2004-12-01

    Environmental indicators can be used as a first stage in progress towards comprehensive environmental impact measures [J. Environ. Manage 65/3 (2002) 285]. In this article, we develop a 'pollutant interaction matrix method' that allows calculation of a global environmental protection index (Ep) in order to verify the eco-compatibility of an industrial activity. Two methods are proposed for the Ep index evaluation (which represents the numerical measure of the environmental sustainability): the Direct Method (Epd) and the Weighted Method (Epw). Both methods need to define, in the whole industrial process, homogeneous sectors (defined as construction sites where activities of the same type are carried out). Furthermore, for each activity a set of parameters (t, duration of pollution effect, P, quantity of pollutant produced,G, hazard of the pollutant) are required to evaluate the relative pollution index Y. All indices calculations were carried out using a set of matrices. The correct use of Ep evaluation provides an improvement in the total environmental performance of companies because it points out possible critical operations in each homogeneous sector which require solutions. The methodology is applied to evaluate the environmental pollution risk of a company that produces polymer materials and to improve their environmental performance. The results obtained show that the whole productive process has a low environmental impact factor. Nevertheless the applied methodology puts in evidence some processes that generate local pollution in specific areas of the factory and which could be dangerous for the workers' health. PMID:15531386

  12. Cosmogenic nuclides application on French Mediterranean shore platform development

    NASA Astrophysics Data System (ADS)

    Giuliano, Jérémy; Lebourg, Thomas; Godard, Vincent; Dewez, Thomas; Braucher, Régis; Bourlès, Didier; Marçot, Nathalie

    2014-05-01

    Rocky shorelines are among the most common elements of the world's littoral zone, and the potential effects of rising sea level on the ever increasing populations require a better understanding of their dynamics. The sinuosity and heterogeneity of the shoreline morphology at large and intermediate wavelengths (1-100 km) results from their constant evolution under the combined influence of marine and continental forcings. This macro-scale organization is the expression of the action of elementary erosion processes acting at shorter wavelengths (<1 km) which lead to the development of shore platforms by landward retreat of cliff edges. Modern analytical techniques (laser-scaning, micro-erosion meters, aerial surveys) constitute appropriate methods to identify and quantify processes of cliff retreat to 1-100 yrs time-scales. But over this time frame, shore platform development appears imperceptible. Precise knowledge of long-term erosion rates are needed to understand rocky shore evolution, and develop quantitative modeling of platform development. Rocky coasts constitute a Quaternary sea level evolution archive that is partly preserved and progressively destroyed. One major challenges is to determine the degree to which coast morphologies are (i) contemporary, (ii) or ancient features inherited, (iii) or partly inherited from Quaternary interglacial stages. In order to fill the lack of long term coast morphodynamic data, we use cosmogenic nuclides (36Cl) to study abrasion surfaces carved in carbonates lithologies along the French Mediterranean coast, in a microtidal environment (Côte Bleue, West of Marseille). 36Cl concentration heritage influences strongly our interpretations in terms of age and denudation of the surfaces. We propose to constrain heritage in sampling oldest relic marine surfaces at 10m of altitude, and along recent cliff scarp. 36Cl concentrations show that the lowest platforms near sea level are contemporary and the highest ones (8-14 m above sea

  13. Composites

    NASA Astrophysics Data System (ADS)

    Taylor, John G.

    The Composites market is arguably the most challenging and profitable market for phenolic resins aside from electronics. The variety of products and processes encountered creates the challenges, and the demand for high performance in critical operations brings value. Phenolic composite materials are rendered into a wide range of components to supply a diverse and fragmented commercial base that includes customers in aerospace (Space Shuttle), aircraft (interiors and brakes), mass transit (interiors), defense (blast protection), marine, mine ducting, off-shore (ducts and grating) and infrastructure (architectural) to name a few. For example, phenolic resin is a critical adhesive in the manufacture of honeycomb sandwich panels. Various solvent and water based resins are described along with resin characteristics and the role of metal ions for enhanced thermal stability of the resin used to coat the honeycomb. Featured new developments include pultrusion of phenolic grating, success in RTM/VARTM fabricated parts, new ballistic developments for military vehicles and high char yield carbon-carbon composites along with many others. Additionally, global regional market resin volumes and sales are presented and compared with other thermosetting resin systems.

  14. Calculated absorption and scattering properties of gold nanoparticles of different size, shape, and composition: applications in biological imaging and biomedicine.

    PubMed

    Jain, Prashant K; Lee, Kyeong Seok; El-Sayed, Ivan H; El-Sayed, Mostafa A

    2006-04-13

    The selection of nanoparticles for achieving efficient contrast for biological and cell imaging applications, as well as for photothermal therapeutic applications, is based on the optical properties of the nanoparticles. We use Mie theory and discrete dipole approximation method to calculate absorption and scattering efficiencies and optical resonance wavelengths for three commonly used classes of nanoparticles: gold nanospheres, silica-gold nanoshells, and gold nanorods. The calculated spectra clearly reflect the well-known dependence of nanoparticle optical properties viz. the resonance wavelength, the extinction cross-section, and the ratio of scattering to absorption, on the nanoparticle dimensions. A systematic quantitative study of the various trends is presented. By increasing the size of gold nanospheres from 20 to 80 nm, the magnitude of extinction as well as the relative contribution of scattering to the extinction rapidly increases. Gold nanospheres in the size range commonly employed ( approximately 40 nm) show an absorption cross-section 5 orders higher than conventional absorbing dyes, while the magnitude of light scattering by 80-nm gold nanospheres is 5 orders higher than the light emission from strongly fluorescing dyes. The variation in the plasmon wavelength maximum of nanospheres, i.e., from approximately 520 to 550 nm, is however too limited to be useful for in vivo applications. Gold nanoshells are found to have optical cross-sections comparable to and even higher than the nanospheres. Additionally, their optical resonances lie favorably in the near-infrared region. The resonance wavelength can be rapidly increased by either increasing the total nanoshell size or increasing the ratio of the core-to-shell radius. The total extinction of nanoshells shows a linear dependence on their total size, however, it is independent of the core/shell radius ratio. The relative scattering contribution to the extinction can be rapidly increased by increasing

  15. Composites

    NASA Astrophysics Data System (ADS)

    Chmielewski, M.; Nosewicz, S.; Pietrzak, K.; Rojek, J.; Strojny-Nędza, A.; Mackiewicz, S.; Dutkiewicz, J.

    2014-11-01

    It is commonly known that the properties of sintered materials are strongly related to technological conditions of the densification process. This paper shows the sintering behavior of a NiAl-Al2O3 composite, and its individual components sintered separately. Each kind of material was processed via the powder metallurgy route (hot pressing). The progress of sintering at different stages of the process was tested. Changes in the microstructure were examined using scanning and transmission electron microscopy. Metal-ceramics interface was clean and no additional phases were detected. Correlation between the microstructure, density, and mechanical properties of the sintered materials was analyzed. The values of elastic constants of NiAl/Al2O3 were close to intermetallic ones due to the volume content of the NiAl phase particularly at low densities, where small alumina particles had no impact on the composite's stiffness. The influence of the external pressure of 30 MPa seemed crucial for obtaining satisfactory stiffness for three kinds of the studied materials which were characterized by a high dense microstructure with a low number of isolated spherical pores.

  16. Constraining Landscape History and Glacial Erosivity Using Paired Cosmogenic Nuclides in Upernavik, Northwest Greenland

    NASA Technical Reports Server (NTRS)

    Corbett, Lee B.; Bierman, Paul R.; Graly, Joseph A.; Neumann, Thomas A.; Rood, Dylan H.

    2013-01-01

    High-latitude landscape evolution processes have the potential to preserve old, relict surfaces through burial by cold-based, nonerosive glacial ice. To investigate landscape history and age in the high Arctic, we analyzed in situ cosmogenic Be(sup 10) and Al (sup 26) in 33 rocks from Upernavik, northwest Greenland. We sampled adjacent bedrock-boulder pairs along a 100 km transect at elevations up to 1000 m above sea level. Bedrock samples gave significantly older apparent exposure ages than corresponding boulder samples, and minimum limiting ages increased with elevation. Two-isotope calculations Al(sup26)/B(sup 10) on 20 of the 33 samples yielded minimum limiting exposure durations up to 112 k.y., minimum limiting burial durations up to 900 k.y., and minimum limiting total histories up to 990 k.y. The prevalence of BE(sup 10) and Al(sup 26) inherited from previous periods of exposure, especially in bedrock samples at high elevation, indicates that these areas record long and complex surface exposure histories, including significant periods of burial with little subglacial erosion. The long total histories suggest that these high elevation surfaces were largely preserved beneath cold-based, nonerosive ice or snowfields for at least the latter half of the Quaternary. Because of high concentrations of inherited nuclides, only the six youngest boulder samples appear to record the timing of ice retreat. These six samples suggest deglaciation of the Upernavik coast at 11.3 +/- 0.5 ka (average +/- 1 standard deviation). There is no difference in deglaciation age along the 100 km sample transect, indicating that the ice-marginal position retreated rapidly at rates of approx.120 m yr(sup-1).

  17. Comparison of RESRAD with hand calculations

    SciTech Connect

    Rittmann, P.D.

    1995-09-01

    This report is a continuation of an earlier comparison done with two other computer programs, GENII and PATHRAE. The dose calculations by the two programs were compared with each other and with hand calculations. These band calculations have now been compared with RESRAD Version 5.41 to examine the use of standard models and parameters in this computer program. The hand calculations disclosed a significant computational error in RESRAD. The Pu-241 ingestion doses are five orders of magnitude too small. In addition, the external doses from some nuclides differ greatly from expected values. Both of these deficiencies have been corrected in later versions of RESRAD.

  18. Fast-neutron activation of long-lived nuclides in natural Pb

    NASA Astrophysics Data System (ADS)

    Guiseppe, V. E.; Elliott, S. R.; Fields, N. E.; Hixon, D.

    2015-04-01

    We measured the production of the long-lived nuclides 207 Bi, 202 Pb, and 194 Hg in a sample of natural Pb due to high-energy neutron interactions using a neutron beam at the Los Alamos Neutron Science Center. The activated sample was counted by a HPGe detector to measure the amount of radioactive nuclides present. These nuclides are critical in understanding potential backgrounds in low background experiments utilizing large amounts of Pb shielding due to cosmogenic neutron interactions in the Pb while residing on the Earth's surface. By scaling the LANSCE neutron flux to a cosmic neutron flux, we measure the sea level cosmic ray production rates of 8.0 ± 1.3 atoms/kg/day of 194 Hg, 120 ± 25 atoms/kg/day 202 Pb, and <0.17 ± 0.04 atoms/kg/day 207 Bi.

  19. (n, charged particle) reactions on lp-shell nuclides at 14 MeV

    SciTech Connect

    Haight, R.C.

    1981-06-01

    The reactions (n,p), (n,d), (n,t) and (n,..cap alpha..) of 14-MeV neutrons with 1p-shell nuclides are of interest in several areas: they can provide tests of charge symmetry by comparisons with proton-induced reactions (on T=O nuclides); they allow study of the complex, often many-body decay of excited nuclear states; and they yield information on final-state interactions. As part of the program in (n, charged particle) reaction studies, several 1p-shell nuclides were investigated: /sup 9/Be, /sup 12/C, /sup 14/N, and /sup 16/O at E/sub n/ = 14 MeV (Haight et. al. 1981). These measurements, with the newly developed magnetic quadrupole charged-particle spectrometer, provide data with a much higher signal-to-background than heretofore available. Experimental methods and results are briefly described. (WHK)

  20. Measuring the noble metal and iodine composition of extracted noble metal phase from spent nuclear fuel using instrumental neutron activation analysis.

    PubMed

    Palomares, R I; Dayman, K J; Landsberger, S; Biegalski, S R; Soderquist, C Z; Casella, A J; Brady Raap, M C; Schwantes, J M

    2015-04-01

    Masses of noble metal and iodine nuclides in the metallic noble metal phase extracted from spent fuel are measured using instrumental neutron activation analysis. Nuclide presence is predicted using fission yield analysis, and radionuclides are identified and the masses quantified using neutron activation analysis. The nuclide compositions of noble metal phase derived from two dissolution methods, UO2 fuel dissolved in nitric acid and UO2 fuel dissolved in ammonium-carbonate and hydrogen-peroxide solution, are compared. PMID:25644079

  1. A model for calculating the errors of 2D bulk analysis relative to the true 3D bulk composition of an object, with application to chondrules

    NASA Astrophysics Data System (ADS)

    Hezel, Dominik C.

    2007-09-01

    Certain problems in Geosciences require knowledge of the chemical bulk composition of objects, such as, for example, minerals or lithic clasts. This 3D bulk chemical composition (bcc) is often difficult to obtain, but if the object is prepared as a thin or thick polished section a 2D bcc can be easily determined using, for example, an electron microprobe. The 2D bcc contains an error relative to the true 3D bcc that is unknown. Here I present a computer program that calculates this error, which is represented as the standard deviation of the 2D bcc relative to the real 3D bcc. A requirement for such calculations is an approximate structure of the 3D object. In petrological applications, the known fabrics of rocks facilitate modeling. The size of the standard deviation depends on (1) the modal abundance of the phases, (2) the element concentration differences between phases and (3) the distribution of the phases, i.e. the homogeneity/heterogeneity of the object considered. A newly introduced parameter " τ" is used as a measure of this homogeneity/heterogeneity. Accessory phases, which do not necessarily appear in 2D thin sections, are a second source of error, in particular if they contain high concentrations of specific elements. An abundance of only 1 vol% of an accessory phase may raise the 3D bcc of an element by up to a factor of ˜8. The code can be queried as to whether broad beam, point, line or area analysis technique is best for obtaining 2D bcc. No general conclusion can be deduced, as the error rates of these techniques depend on the specific structure of the object considered. As an example chondrules—rapidly solidified melt droplets of chondritic meteorites—are used. It is demonstrated that 2D bcc may be used to reveal trends in the chemistry of 3D objects.

  2. Applications of in situ cosmogenic nuclides in the geologic site characterization of Yucca Mountain, Nevada

    SciTech Connect

    Gosse, J.C.; Harrington, C.D.; Whitney, J.W.

    1995-12-31

    The gradual buildup of rare isotopes from interactions between cosmic rays and atoms in an exposed rock provides a new method of directly determining the exposure age of rock surfaces. The cosmogenic nuclide method can also provide constraints on erosion rates and the length of time surface exposure was interrupted by burial. Numerous successful applications of the technique have been imperative to the complete surface geologic characterization of Yucca Mountain, Nevada, a potential high level nuclear waste repository. In this short paper, we summarize the cosmogenic nuclide method and describe with examples some the utility of the technique in geologic site characterization. We report preliminary results from our ongoing work at Yucca Mountain.

  3. Reprocessing system with nuclide separation based on chromatography in hydrochloric acid solution

    SciTech Connect

    Suzuki, Tatsuya; Tachibana, Yu; Koyama, Shi-ichi

    2013-07-01

    We have proposed the reprocessing system with nuclide separation processes based on the chromatographic technique in the hydrochloric acid solution system. Our proposed system consists of the dissolution process, the reprocessing process, the minor actinide separation process, and nuclide separation processes. In the reprocessing and separation processes, the pyridine resin is used as a main separation media. It was confirmed that the dissolution in the hydrochloric acid solution is easily achieved by the plasma voloxidation and by the addition of oxygen peroxide into the hydrochloric acid solution.

  4. Apparatus and method for quantitatively evaluating total fissile and total fertile nuclide content in samples

    DOEpatents

    Caldwell, John T.; Kunz, Walter E.; Cates, Michael R.; Franks, Larry A.

    1985-01-01

    Simultaneous photon and neutron interrogation of samples for the quantitative determination of total fissile nuclide and total fertile nuclide material present is made possible by the use of an electron accelerator. Prompt and delayed neutrons produced from resulting induced fissions are counted using a single detection system and allow the resolution of the contributions from each interrogating flux leading in turn to the quantitative determination sought. Detection limits for .sup.239 Pu are estimated to be about 3 mg using prompt fission neutrons and about 6 mg using delayed neutrons.

  5. 26Al - 10Be cosmogenic nuclide isochron burial dating in combination with luminescence dating of two Danube terraces

    NASA Astrophysics Data System (ADS)

    Neuhuber, Stephanie; Braumann, Sandra; Lüthgens, Christopher; Fiebig, Markus; Häuselmann, Philipp; Schäfer, Jörg

    2016-04-01

    The Quaternary sediment record in the Vienna Basin is influenced by two main factors: (1) the tectonic development of a pull apart basin along a sinistral strike slip fault system between the Eastern Alps and the West Carpathians and by (2) strongly varying sediment supply during the Plio- and Pleistocene. From the Late Pannonian (8.8 Ma) onward a large-scale regional uplift (Decker et al., 2005) controls terrace formation in the Vienna Basin. The main sediment supply into the Vienna Basin originates from the Danube, and subordinately from tributaries to the south such as Piesting, Fischa, Leitha and from the north by the river March. Today the Danube forms a large floodplain that is bordered to the north by one large Pleistocene terrace, the Gänserndorf Terrace that is situated 17 m above todays water level. Farther to the east a smaller terrace, the Schlosshof Terrace, reaches 25 m above todays water level. These terrace levels are tilted by movement of underlying blocks (Peresson, 2006). Both, the Schlosshof and Gänserndorf terraces consist of successions of up to 2 m thick gravel beds with intercalated sand layers or -lenses that may locally reach thicknesses up to 0.8 m. At each terrace one gavel pit was selected to calculate the time of terrace deposition by luminescence dating in combination with 26Al/10Be cosmogenic nuclide isochrone dating (Balco and Rovery, 2008). Five quartz stones from the base of each terrace were physically and chemically processed to obtain Al and Be oxides for Acceleration Mass Spectrometry. Sand samples for luminescence dating were taken above the cosmogenic nuclide samples from the closest suitable sand body. Decker et al., 2005. QSR 24, 307-322 Peresson, 2006 Geologie der österreichischen Bundesländer Niederösterreich 255-258 Balco and Rovey, 2008. AJS 908, 1083-1114 Thanks to FWF P 23138-N19, OMAA 90öu17

  6. A Method for Calculating Strain Energy Release Rates in Preliminary Design of Composite Skin/Stringer Debonding Under Multi-Axial Loading

    NASA Technical Reports Server (NTRS)

    Krueger, Ronald; Minguet, Pierre J.; OBrien, T. Kevin

    1999-01-01

    Three simple procedures were developed to determine strain energy release rates, G, in composite skin/stringer specimens for various combinations of unaxial and biaxial (in-plane/out-of-plane) loading conditions. These procedures may be used for parametric design studies in such a way that only a few finite element computations will be necessary for a study of many load combinations. The results were compared with mixed mode strain energy release rates calculated directly from nonlinear two-dimensional plane-strain finite element analyses using the virtual crack closure technique. The first procedure involved solving three unknown parameters needed to determine the energy release rates. Good agreement was obtained when the external loads were used in the expression derived. This superposition technique was only applicable if the structure exhibits a linear load/deflection behavior. Consequently, a second technique was derived which was applicable in the case of nonlinear load/deformation behavior. The technique involved calculating six unknown parameters from a set of six simultaneous linear equations with data from six nonlinear analyses to determine the energy release rates. This procedure was not time efficient, and hence, less appealing. A third procedure was developed to calculate mixed mode energy release rates as a function of delamination lengths. This procedure required only one nonlinear finite element analysis of the specimen with a single delamination length to obtain a reference solution for the energy release rates and the scale factors. The delamination was extended in three separate linear models of the local area in the vicinity of the delamination subjected to unit loads to obtain the distribution of G with delamination lengths. This set of sub-problems was Although additional modeling effort is required to create the sub- models, this local technique is efficient for parametric studies.

  7. Development of Advanced Nuclide Separation and Recovery Methods using Ion-Exchanhge Techniques in Nuclear Backend

    NASA Astrophysics Data System (ADS)

    Miura, Hitoshi

    The development of compact separation and recovery methods using selective ion-exchange techniques is very important for the reprocessing and high-level liquid wastes (HLLWs) treatment in the nuclear backend field. The selective nuclide separation techniques are effective for the volume reduction of wastes and the utilization of valuable nuclides, and expected for the construction of advanced nuclear fuel cycle system and the rationalization of waste treatment. In order to accomplish the selective nuclide separation, the design and synthesis of novel adsorbents are essential for the development of compact and precise separation processes. The present paper deals with the preparation of highly functional and selective hybrid microcapsules enclosing nano-adsorbents in the alginate gel polymer matrices by sol-gel methods, their characterization and the clarification of selective adsorption properties by batch and column methods. The selective separation of Cs, Pd and Re in real HLLW was further accomplished by using novel microcapsules, and an advanced nuclide separation system was proposed by the combination of selective processes using microcapsules.

  8. The intercomparison of mixed nuclide rod source sets used to calibrate waste assay systems

    SciTech Connect

    Kirkpatrick, J.M.; Philips, S.; Croft, S.

    2007-07-01

    The relative activities of five sets of commercially available, certified mixed-nuclide rod gamma sources have been measured. The results are compared with one another and with the manufacturer's calibration certificates in order to evaluate the self consistency, accuracies and uncertainties of the activities claimed. The comparison measurements were made with Canberra's Tomographic Gamma Scanner (TGS) System in Segmented Gamma Scanner (SGS) mode, operated with a single segment and using a 120% relative efficiency HPGe detector. Each set of six rods was measured in a rotating 208-liter drum geometry typical of applications in which such rod source sets are commonly used for both initial calibration and operational verification measurements. Three of the five source sets were found to be consistent with one another within the experimental and claimed certificate uncertainties; however, two of the mixed-nuclide source sets were found to have nuclide-to-nuclide variations of activity significantly in excess of expectations based upon the claimed 99% confidence-level uncertainties. Such discrepancies could introduce substantial bias into waste measurement results made using the afflicted rod sets as the calibration standards. The findings of this work lead us to conclude that, where possible, the certified activities and associated uncertainties on newly acquired sources should be independently confirmed before relying on them as calibration standards. (authors)

  9. An improved choice of oscillator basis for banana shaped nuclides

    SciTech Connect

    Chasman, R.R.

    1994-03-01

    The question of the appropriate choice of oscillator basis functions for studying exotic nuclear shapes is raised. Difficulties with the conventional choice of oscillator basis states are noted for shapes having a large banana component. A prescription for an improved oscillator basis to study these shapes is given. It can be applied in a more general context. New calculations with this improved basis are presented for the banana deformation mode. The change of basis gives results that improve the prospects of finding states in the banana minimum for many isotopes of Tl, Pb and Bi.

  10. Optical model methods of predicting nuclide production from spallation reactions

    NASA Technical Reports Server (NTRS)

    Ramsey, C. R.; Townsend, L. W.; Tripathi, R. K.; Cucinotta, F. A.; Wilson, J. W. (Principal Investigator)

    1998-01-01

    Quantum mechanical optical model methods for calculating isotope production cross sections from the spallation of heavy nuclei by high-energy protons are developed from a modified abrasion-ablation collision formalism. The abrasion step is treated quantum-mechanically as a knockout process which leaves the residual prefragment nucleus in an excited state. In ablation the prefragment deexcites to produce the final fragment. The excitation energies of the prefragments are estimated from a combination of liquid drop and frictional-spectator interaction considerations. Estimates of elemental and isotopic production cross sections are in good agreement with recently published cross section measurements.

  11. Using Cosmogenic Nuclides to Examine Erosional Steady-State in the Western Alps

    NASA Astrophysics Data System (ADS)

    Perg, L. A.; von Blanckenburg, F.; Kubik, P.

    2002-12-01

    Geomorphologists have long been interested in the amount of time needed for landscapes to reach equilibrium after climate or tectonic perturbation. Cosmogenic nuclides provide a means to determine whether landscapes have reached equilibrium after glacial retreat. The cosmogenic nuclide budget should be mostly balanced (input through production equals output through erosion) after removal of one spallation length scale, about 60 cm of material. If a catchment has achieved steady-state erosional loss of cosmogenic nuclides, the cosmogenic nuclide concentration of the river sediment will provide the long-term basin-averaged denudation rate. If a deglaciated catchment has not reached steady-state, the apparent erosion rates will be too high. The apparent erosion rates obtained using cosmogenic nuclides can be compared with the denudation rates obtained from sediment accumulation in glacial lakes and valleys to determine whether the landscape has reached steady-state. Different sediment sources were sampled along a NS transect through the Western Alps from the highland (1 mm/yr uplift) to the foreland (no uplift, net deposition). Samples include: subglacial outwash; intraglacial sediment; moraines (surface and deeply buried material); currently glaciated, formerly glaciated and never glaciated catchments; and large river samples that integrate these sediment sources. Sediment traps indicate a long-term erosion rate of about 0.12 m / k.y. in the W. Alps during the Holocene (Hinderer, 2001). At this rate of denudation, the cosmogenic nuclide concentrations should approach steady-state in 5-6 k.y. However, the apparent cosmogenic nuclide erosion rates are much higher (0.3 m / k.y. in the foreland and 2 m / k.y. in the highland) indicating that the landscape has not reached equilibrium in two to three times that length of time. One possible explanation is intermediate sediment storage, such as alluvial fans, with higher concentration sediment not yet reaching the streams

  12. The light curve of SN 1987A revisited: constraining production masses of radioactive nuclides

    SciTech Connect

    Seitenzahl, Ivo R.; Timmes, F. X.; Magkotsios, Georgios

    2014-09-01

    We revisit the evidence for the contribution of the long-lived radioactive nuclides {sup 44}Ti, {sup 55}Fe, {sup 56}Co, {sup 57}Co, and {sup 60}Co to the UVOIR light curve of SN 1987A. We show that the V-band luminosity constitutes a roughly constant fraction of the bolometric luminosity between 900 and 1900 days, and we obtain an approximate bolometric light curve out to 4334 days by scaling the late time V-band data by a constant factor where no bolometric light curve data is available. Considering the five most relevant decay chains starting at {sup 44}Ti, {sup 55}Co, {sup 56}Ni, {sup 57}Ni, and {sup 60}Co, we perform a least squares fit to the constructed composite bolometric light curve. For the nickel isotopes, we obtain best fit values of M({sup 56}Ni) = (7.1 ± 0.3) × 10{sup –2} M {sub ☉} and M({sup 57}Ni) = (4.1 ± 1.8) × 10{sup –3} M {sub ☉}. Our best fit {sup 44}Ti mass is M({sup 44}Ti) = (0.55 ± 0.17) × 10{sup –4} M {sub ☉}, which is in disagreement with the much higher (3.1 ± 0.8) × 10{sup –4} M {sub ☉} recently derived from INTEGRAL observations. The associated uncertainties far exceed the best fit values for {sup 55}Co and {sup 60}Co and, as a result, we only give upper limits on the production masses of M({sup 55}Co) < 7.2 × 10{sup –3} M {sub ☉} and M({sup 60}Co) < 1.7 × 10{sup –4} M {sub ☉}. Furthermore, we find that the leptonic channels in the decay of {sup 57}Co (internal conversion and Auger electrons) are a significant contribution and constitute up to 15.5% of the total luminosity. Consideration of the kinetic energy of these electrons is essential in lowering our best fit nickel isotope production ratio to [{sup 57}Ni/{sup 56}Ni] = 2.5 ± 1.1, which is still somewhat high but is in agreement with gamma-ray observations and model predictions.

  13. A model for the production of cosmogenic nuclides in chondrites

    NASA Technical Reports Server (NTRS)

    Graf, TH.; Baur, H.; Signer, P.

    1990-01-01

    A model is presented for calculating the production rates of cosmic-ray-produced He, Ne, and Ar as well as Be-10, Al-26, and Mn-53 in chondrites of variable size and shape. The predictions of this model are compared with published data for the meteorites ALH78084, St. Severin, and Keyes. The agreement is found to be about 5 percent for the concentrations of Be-10, Ne-21, Ne-22, Ar-38, and Mn-53, and to be better than 1 percent for the Ne-22/Ne-21 ratios. The correlation between P(Be-10)/P(Ne-21) and Ne-22/Ne-21 ratios is experimentally verified over a wide range of irradiation conditions.

  14. Kinetics analysis and quantitative calculations for the successive radioactive decay process

    NASA Astrophysics Data System (ADS)

    Zhou, Zhiping; Yan, Deyue; Zhao, Yuliang; Chai, Zhifang

    2015-01-01

    The general radioactive decay kinetics equations with branching were developed and the analytical solutions were derived by Laplace transform method. The time dependence of all the nuclide concentrations can be easily obtained by applying the equations to any known radioactive decay series. Taking the example of thorium radioactive decay series, the concentration evolution over time of various nuclide members in the family has been given by the quantitative numerical calculations with a computer. The method can be applied to the quantitative prediction and analysis for the daughter nuclides in the successive decay with branching of the complicated radioactive processes, such as the natural radioactive decay series, nuclear reactor, nuclear waste disposal, nuclear spallation, synthesis and identification of superheavy nuclides, radioactive ion beam physics and chemistry, etc.

  15. ANEMOS: A computer code to estimate air concentrations and ground deposition rates for atmospheric nuclides emitted from multiple operating sources

    SciTech Connect

    Miller, C.W.; Sjoreen, A.L.; Begovich, C.L.; Hermann, O.W.

    1986-11-01

    This code estimates concentrations in air and ground deposition rates for Atmospheric Nuclides Emitted from Multiple Operating Sources. ANEMOS is one component of an integrated Computerized Radiological Risk Investigation System (CRRIS) developed for the US Environmental Protection Agency (EPA) for use in performing radiological assessments and in developing radiation standards. The concentrations and deposition rates calculated by ANEMOS are used in subsequent portions of the CRRIS for estimating doses and risks to man. The calculations made in ANEMOS are based on the use of a straight-line Gaussian plume atmospheric dispersion model with both dry and wet deposition parameter options. The code will accommodate a ground-level or elevated point and area source or windblown source. Adjustments may be made during the calculations for surface roughness, building wake effects, terrain height, wind speed at the height of release, the variation in plume rise as a function of downwind distance, and the in-growth and decay of daughter products in the plume as it travels downwind. ANEMOS can also accommodate multiple particle sizes and clearance classes, and it may be used to calculate the dose from a finite plume of gamma-ray-emitting radionuclides passing overhead. The output of this code is presented for 16 sectors of a circular grid. ANEMOS can calculate both the sector-average concentrations and deposition rates at a given set of downwind distances in each sector and the average of these quantities over an area within each sector bounded by two successive downwind distances. ANEMOS is designed to be used primarily for continuous, long-term radionuclide releases. This report describes the models used in the code, their computer implementation, the uncertainty associated with their use, and the use of ANEMOS in conjunction with other codes in the CRRIS. A listing of the code is included in Appendix C.

  16. Nuclide Importance to Criticality Safety, Decay Heating, and Source Terms Related to Transport and Interim Storage of High-Burnup LWR Fuel

    SciTech Connect

    Gauld, I. C.; Ryman, J. C.

    2000-12-11

    This report investigates trends in the radiological decay properties and changes in relative nuclide importance associated with increasing enrichments and burnup for spent LWR fuel as they affect the areas of criticality safety, thermal analysis (decay heat), and shielding analysis of spent fuel transport and storage casks. To facilitate identifying the changes in the spent fuel compositions that most directly impact these application areas, the dominant nuclides in each area have been identified and ranked by importance. The importance is investigated as a function of increasing burnup to assist in identifying the key changes in spent fuel characteristics between conventional- and extended-burnup regimes. Studies involving both pressurized water-reactor (PWR) fuel assemblies and boiling-water-reactor (BWR) assemblies are included. This study is seen to be a necessary first step in identifying the high-burnup spent fuel characteristics that may adversely affect the accuracy of current computational methods and data, assess the potential impact on previous guidance on isotopic source terms and decay-heat values, and thus help identify areas for methods and data improvement. Finally, several recommendations on the direction of possible future code validation efforts for high-burnup spent fuel predictions are presented.

  17. Weathering histories of Chinese loess deposits based on uranium and thorium series nuclides and cosmogenic {sup 10}Be

    SciTech Connect

    Gu, Z.Y. |; Lal, D.; Liu, T.S.

    1997-12-01

    The long, continuous deposition of dust in the Chinese loess plateau offers an unique opportunity to study the nature of soil weathering in a wide range of climatic conditions. In this paper we report on measurements of concentrations of U- and Th-series nuclides and of major cations in 150 loess and paleosol samples from five sites, going back 2.5 Ma. Using the results for {sup 10}Be concentrations in these soils, we determined the absolute amounts of water added to several soil units and obtained: (1) first-order leaching constants for U and several cations and (2) the compositions of the soils contributing to the dust-source regions and of the dust at deposition. Further, based on analyses of {sup 230}Th in soils deposited in the past ca. 140 ka, we determined when the soils weathered in the source regions. We conclude that most of the weathering in the dust-source regions may have occurred during the interglacials. 34 refs., 8 figs., 2 tabs.

  18. The production of residual nuclides in Pb irradiated by 400 MeV/u carbon ions

    NASA Astrophysics Data System (ADS)

    Ge, H. L.; Ma, F.; Zhang, X. Y.; Ju, Y. Q.; Zhang, H. B.; Chen, L.; Luo, P.; Zhou, B.; Zhang, Y. B.; Li, J. Y.; Xu, J. K.; Liang, T. J.; Wang, S. L.; Yang, Y. W.; Yang, L.

    2014-10-01

    The experiment was performed by irradiating a Pb foil with 400 MeV/u carbon beam at the HIRFL-CSR in Lanzhou, China. The experimental data was acquired by the off-line γ-spectroscopy method. 32 radioactive residual nuclides had been observed and their cross sections were determined. The measured results were compared with the results simulated by Monte Carlo code MCNPX2.7.0. The comparison shows that the simulated cross sections were underestimated for the fragments from A = 20 to 41 and A = 110 to 175. By fitting the measured and simulated cross sections to Rudstams semi-empirical formula, it was found that the charge distribution of products was asymmetric for the residual nuclides with a high mass number.

  19. Determination of Concentrations of Radioactive Nuclides in Soil Samples using Gamma Ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Adil, Arsalan; Weaver, Joshua

    2015-10-01

    A hyper-pure Germanium detector system was used to determine the contents and concentrations of various nuclides in soil samples collected from different parts of the United States. These include areas in close proximity to nuclear power plants, areas susceptible to nuclear fallout from weapons testing from the pre Comprehensive Nuclear Test Ban Treaty (CTBT) period, and areas vulnerable to fallout from Fukushima from the west coast. The concentrations of naturally occurring nuclides in the 238U, 232Th, and 40K decay chains as well as that of synthetic isotopes of 137Cs and 60Co were measured with the aid of Genie-2000 and Radware (gf3m). An efficiency curve was obtained by designing a simulation and compared with standard sources. The research, now in its next stage, aims to do the same in samples from Karachi (Pakistan) which is home to three nuclear power plant projects but has no available baseline radioactivity measurements. University of Richmond.

  20. The exposure history of Jilin and production rates of cosmogenic nuclides

    NASA Technical Reports Server (NTRS)

    Heusser, G.

    1986-01-01

    Jilin, the largest known story meteorite, is a very suitable object for studying the systematics of cosmic ray produced nuclides in stony meteorites. Its well established two stage exposure history even permits to gain information about two different irradiation geometries (2pi and 4pi). All stable and long-lived cosmogenic nuclides measured in Jilin so far correlate well with each other. An example is shown where the Al-26 activities are plotted vs. the spallogenic Ne-21 concentration. These records of cosmic-ray interaction in Jilin can be used both to determine the history of the target and to study the nature of production rate profiles. This is unavoidably a bootstrap process, involving studying one with assumption about the other. Production rate equations are presented and discussed.

  1. Heavy mass elements total half-lives for selected long-lived nuclides

    SciTech Connect

    Holden, N.E.

    1985-01-01

    In the past, many compilations and evaluations of half-lives have been made which have uncritically accepted authors' values and uncertainties. They have merely recommended weight-averaged reported results. This evaluation attempts to reanalyze each experiment in the literature including an estimate of the standard deviation utilizing, where possible, an estimate of the systematic error. This paper constitutes a preliminary step in the process of recommending values. The long-lived nuclides of heavy mass elements are of interest in determining geological ages using the Re-Os or the Lu-Hf dating methods, in supplying information on the p-process (proton capture) of nucleo-synthesis, in providing information on lepton number conservation and the rest mass for the electron neutrino from double ..beta.. decay processes and in the case of tantalum because it represents the first long-lived state which is actually an isomer. Experimental data on the half-lives of selected nuclides have been evaluated and recommended values and uncertainties are presented for the following nuclides: /sup 128/Te, /sup 130/Te, /sup 129/I, /sup 138/La, /sup 144,145/Nd, /sup 146,147,148/Sm, /sup 152/Gd, /sup 154/Dy, /sup 176/Lu, /sup 174/Hf, /sup 180/Ta, /sup 187/Re, /sup 186/Os, /sup 190/Pt, /sup 204,205/Pb and /sup 230,232/Th. It is shown that /sup 204/Pb, which was previously thought to be radioactive, is stable. For /sup 205/Pb, the L electron capture x-rays have been revised for the M and higher x-ray yields. The resulting half-life for /sup 205/Pb is 1.9 +- 0.3 x 10/sup 7/ years. /sup 146/Sm with a half-life of 1.03 +- 0.05 x 10/sup 8/ years is the longest-lived extinct natural nuclide. 21 tabs.

  2. NHEXAS PHASE I ARIZONA STUDY--STANDARD OPERATING PROCEDURE FOR CALCULATING INGESTION EXPOSURE FROM DAY 4 COMPOSITE MEASUREMENTS, THE DIRECT METHOD OF EXPOSURE ESTIMATION (IIT-A-6.0)

    EPA Science Inventory

    The purpose of this SOP is to describe the procedures undertaken for calculating ingestion exposure from Day 4 composite measurements from duplicate diet using the direct method of exposure estimation. This SOP uses data that have been properly coded and certified with appropria...

  3. REVIEW OF RESULTS FOR THE OECD/NEA PHASE VII BENCHMARK: STUDY OF SPENT FUEL COMPOSITIONS FOR LONG TERM DISPOSAL

    SciTech Connect

    Radulescu, Georgeta; Wagner, John C

    2011-01-01

    This paper summarizes the problem specification and compares participants results for the OECD/NEA/WPNCS Expert Group on Burn-up Credit Criticality Safety Phase VII Benchmark Study of Spent Fuel Compositions for Long-Term Disposal. The Phase VII benchmark was developed to study the ability of relevant computer codes and associated nuclear data to predict spent fuel isotopic compositions and corresponding keff values in a cask configuration over the time duration relevant to spent nuclear fuel (SNF) disposal. The benchmark was divided into two sets of calculations: (1) decay calculations out to 1,000,000 years for provided pressurized-water-reactor (PWR) UO2 discharged fuel compositions and (2) burnup credit criticality calculations for a representative cask model at selected time steps. Contributions from 15 organizations and companies in 10 countries were submitted to the Phase VII benchmark exercise. This paper provides a description of the Phase VII benchmark and detailed comparisons of the participants isotopic compositions and keff values that were calculated with a diversity of computer codes and nuclear data sets. Differences observed in the calculated time-dependent nuclide densities are attributed to different decay data or code-specific numerical approximations. The variability of the keff results is consistent with the evaluated uncertainty associated with cross-section data.

  4. Fukushima-derived fission nuclides monitored around Taiwan: Free tropospheric versus boundary layer transport

    NASA Astrophysics Data System (ADS)

    Huh, Chih-An; Hsu, Shih-Chieh; Lin, Chuan-Yao

    2012-02-01

    The 2011 Fukushima nuclear accident in Japan was the worst nuclear disaster following the 1986 Chernobyl accident. Fission products (nuclides) released from the Fukushima plant site since March 12, 2011 had been detected around the northern hemisphere in about two weeks and also in the southern hemisphere about one month later. We report here detailed time series of radioiodine and radiocesium isotopes monitored in a regional network around Taiwan, including one high-mountain and three ground-level sites. Our results show several pulses of emission from a sequence of accidents in the Fukushima facility, with the more volatile 131I released preferentially over 134Cs and 137Cs at the beginning. In the middle of the time series, there was a pronounced peak of radiocesium observed in northern Taiwan, with activity concentrations of 134Cs and 137Cs far exceeding that of 131I during that episode. From the first arrival time of these fission nuclides and their spatial and temporal variations at our sampling sites and elsewhere, we suggest that Fukushima-derived radioactive nuclides were transported to Taiwan and its vicinity via two pathways at different altitudes. One was transported in the free troposphere by the prevailing westerly winds around the globe; the other was transported in the planetary boundary layer by the northeast monsoon wind directly toward Taiwan.

  5. Grain size bias in cosmogenic nuclide studies of stream sediment in steep terrain

    NASA Astrophysics Data System (ADS)

    Lukens, Claire E.; Riebe, Clifford S.; Sklar, Leonard S.; Shuster, David L.

    2016-05-01

    Cosmogenic nuclides in stream sediment are widely used to quantify catchment-average erosion rates. A key assumption is that sampled sediment is representative of erosion from the entire catchment. Here we show that the common practice of collecting a narrow range of sizes—typically sand—may not yield a representative sample when the grain size distribution of sediment produced on slopes is spatially variable. A grain size bias arises when some parts of the catchment produce sand more readily than others. To identify catchments that are prone to this bias, we used a forward model of sediment mixing and erosion to explore the effects of catchment relief and area across a range of altitudinal gradients in sediment size and erosion rate. We found that the bias increases with increasing relief, because higher-relief catchments have a larger fraction of high elevations that are underrepresented in the sampled sand when grain size increases with altitude. The bias also increases with catchment area, because sediment size reduction during transport causes an underrepresentation of more distal, higher elevations within the catchment. Our analysis indicates that grain size bias may be significant at many sites where cosmogenic nuclides have been used to quantify catchment-average erosion rates. We discuss how to quantify and account for the bias using cosmogenic nuclides and detrital thermochronometry in multiple sediment sizes.

  6. Light nuclides produced in the proton-induced spallation of {sup 238}U at 1 GeV

    SciTech Connect

    Ricciardi, M.V.; Armbruster, P.; Enqvist, T.; Kelic, A.; Rejmund, F.; Schmidt, K.-H.; Yordanov, O.; Benlliure, J.; Pereira, J.; Bernas, M.; Mustapha, B.; Stephan, C.; Tassan-Got, L.

    2006-01-15

    The production of light and intermediate-mass nuclides formed in the reaction {sup 1}H+{sup 238}U at 1 GeV was measured at the Fragment Separator at GSI, Darmstadt. The experiment was performed in inverse kinematics, by shooting a 1 A GeV {sup 238}U beam on a thin liquid-hydrogen target. A total of 254 isotopes of all elements in the range 7{<=}Z{<=}37 were unambiguously identified, and the velocity distributions of the produced nuclides were determined with high precision. The results show that the nuclides are produced in a very asymmetric binary decay of heavy nuclei originating from the spallation of uranium. All the features of the produced nuclides merge with the characteristics of the fission products as their mass increases.

  7. Long- and short-lived nuclide constraints on the recent evolution of permafrost soils

    NASA Astrophysics Data System (ADS)

    Bagard, M.; Chabaux, F. J.; Rihs, S.; Pokrovsky, O. S.; Prokushkin, A. S.; Viers, J.

    2011-12-01

    Frozen permafrost ecosystems are particularly sensitive to climate warming, which notably induces a deepening of the active layer (the maximum thawing depth during summer time). As a consequence, geochemical and hydrological fluxes within boreal areas are expected to be significantly affected in the future. Understanding the relationship between environmental changes and permafrost modifications is then a major challenge. This work aims to evaluate in a Siberian watershed the dynamics of the permafrost active layer and their recent modifications by combining a classic study of long-lived nuclides to the study of short-lived nuclides of U and Th decay series. Two soil profiles, located on opposite slopes (north- and south-facing slopes) of the Kulingdakan watershed (Putorana Plateau, Central Siberia), were sampled at several depths within the active layer and (238U), (234U), (232Th), (230Th), (226Ra), (228Ra), (228Th) and (210Pb) were measured on bulk soil samples by TIMS or gamma spectrometry. Our results show that south-facing and north-facing soil profiles are significantly different in terms of evolution of chemical concentrations and nuclide activities; north-facing soil profile is strongly affected by atmospheric inputs whereas long-lived nuclide dynamics within south-facing soil profile are dominated by weathering and exhibit more complex patterns. The amount of above-ground biomass being the single varying parameter between the two slopes of the watershed, we suggest that the structuring of permafrost active layer is very sensitive to vegetation activity and that the functioning of boreal soils will be significantly modified by its development due to more favorable climatic conditions. Moreover, the coupling of long and short-lived nuclides highlights the superimposition of a recent mobilization of chemical elements within soils (<10 years) over a much older soil structure (>8000 years), which can be observed for both soil profiles. The shallowest layer of

  8. Recent evolution of permafrost soils: insight from U-Th series nuclides

    NASA Astrophysics Data System (ADS)

    Bagard, marie-laure; Chabaux, Francois; Rihs, Sophie; Pokrovsky, Oleg; Viers, Jérome

    2015-04-01

    Permafrost ecosystems are particularly sensitive to climate warming, which notably induces a deepening of the active layer (the maximum thawing depth during summer time). As a consequence, geochemical and hydrological fluxes within boreal areas are expected to be significantly affected in the future. Understanding the relationship between environmental changes and permafrost modifications is then a major challenge. This work aims to evaluate in a Siberian watershed the dynamics of the permafrost active layer and their recent modifications by combining a classic study of long-lived nuclides to the study of short-lived nuclides of U and Th decay series in two soil profiles. These profiles, located on opposite slopes (north- and south-facing slopes) of the Kulingdakan watershed (Putorana Plateau, Central Siberia), were sampled at several depths within the active layer and (238U), (230Th), (232Th), (226Ra), (228Ra), (228Th), (210Pb) were measured on bulk soil samples by TIMS or gamma spectrometry. Our results show that south-facing and north-facing soil profiles are significantly different in terms of evolution of chemical concentrations and nuclide activities; north-facing soil profile is strongly affected by atmospheric inputs whereas long-lived nuclide dynamics within south-facing soil profile are dominated by weathering and exhibit more complex patterns. The amount of above-ground biomass being the single varying parameter between the two slopes of the watershed, we suggest that the structuring of permafrost active layer is very sensitive to vegetation activity and that the functioning of boreal soils will be significantly modified by its development due to more favorable climatic conditions. Moreover, the coupling of long and short-lived nuclides highlights the superimposition of a recent mobilization of chemical elements within soils (<10 years) over a much older soil structuring (>8000 years), which can be observed for both soil profiles. The shallowest layer of

  9. Nuclear event zero-time calculation and uncertainty evaluation.

    PubMed

    Pan, Pujing; Ungar, R Kurt

    2012-04-01

    It is important to know the initial time, or zero-time, of a nuclear event such as a nuclear weapon's test, a nuclear power plant accident or a nuclear terrorist attack (e.g. with an improvised nuclear device, IND). Together with relevant meteorological information, the calculated zero-time is used to help locate the origin of a nuclear event. The zero-time of a nuclear event can be derived from measured activity ratios of two nuclides. The calculated zero-time of a nuclear event would not be complete without an appropriately evaluated uncertainty term. In this paper, analytical equations for zero-time and the associated uncertainty calculations are derived using a measured activity ratio of two nuclides. Application of the derived equations is illustrated in a realistic example using data from the last Chinese thermonuclear test in 1980. PMID:22305002

  10. Impact of vegetation change on the mobility of uranium- and thorium-series nuclides in soils

    NASA Astrophysics Data System (ADS)

    Gontier, A.; Rihs, S.; Turpault, M.-P.; Chabaux, F.

    2012-04-01

    The effect of land cover change on chemical mobility and soil response was investigated using short- and long-lived nuclides from the U- and Th series. Indeed, the matching of these nuclides half-live to the pedogenic processes rates make these nuclides especially suitable to investigate either time or mechanism of transfers within a soil-water-plant system. This study was carried out from the experimental Breuil-Chenue site (Morvan mountains, France). The native forest (150 year-old) was partially clear-felled and replaced in 1976 by mono-specific plantations distributed in different stands. Following this cover-change, some mineralogical changes in the acid brown soil were recognized (Mareschal, 2008). Three soil sections were sampled under the native forest and the replanted oak and Douglas spruce stands respectively. The (238U), (234U), (230Th), (226Ra), (232Th) and (228Ra) activities were analysed by thermal ionization mass spectrometry (TIMS), inductively coupled plasma mass spectrometry (MC-ICPMS) and gamma spectrometry. Significant differences in U, Th, and Ra activities were observed between the soils located under the native forest or the replanted-trees stands, mostly dominated by a large uranium mobilization from the replanted soils. Moreover, all the investigated U and Th-series activity ratios show a contrasted trend between the shallowest horizons (0-50cm) and the deepest one (below 50cm), demonstrating the chemical effect of the vegetation change on the shallow soil layers. Using a continuous open-system leaching model, the coupled radioactive disequilibria measured in the different soil layers permit to quantify the rate of the radionuclides mobilities. Reference: Mareschal, L., 2008. Effet des substitutions d'essences forestières sur l'évolution des sols et de leur minéralogie : bilan après 28 ans dans le site expérimental de Breuil (Morvan) Université Henri Poincaré, Nancy-I.

  11. Results of calculations of external gamma radiation exposure rates from local fallout and the related radionuclide compositions of two hypothetical 1-MT nuclear bursts. Final report

    SciTech Connect

    Hicks, H.

    1984-12-01

    This report presents data on calculated gamma radiation exposure rates and local surface deposition of related radionuclides resulting from two hypothetical 1-Mt nuclear bursts. Calculations are made of the debris from two types of bombs: one containing /sup 235/U as a fissionable material (designated oralloy), the other containing /sup 238/U (designated tuballoy). 4 references.

  12. Tantalum-178--a short-lived nuclide for nuclear medicine: development of a potential generator system.

    PubMed

    Neirinckx, R D; Jones, A G; Davis, M A; Harris, G I; Holman, B L

    1978-05-01

    We describe a chemical separation that may form the basis of a generator system for the short-lived radionuclide Ta-178 (T 1/2 = 9 min). The parent nuclide W-178 (T 1/2 = 21.7 days) is loaded on an anion-exchange column and the daughter eluted with a mixture of dilute hydrochloric acid and hydrogen peroxide. The yields of tantalum and the breakthrough of the tungsten parent as a function of the eluting conditions are discussed, and preliminary animal distribution data are presented for various treatments of the eluant solution. PMID:641574

  13. Linear Transformation Method for Multinuclide Decay Calculation

    SciTech Connect

    Ding Yuan

    2010-12-29

    A linear transformation method for generic multinuclide decay calculations is presented together with its properties and implications. The method takes advantage of the linear form of the decay solution N(t) = F(t)N{sub 0}, where N(t) is a column vector that represents the numbers of atoms of the radioactive nuclides in the decay chain, N{sub 0} is the initial value vector of N(t), and F(t) is a lower triangular matrix whose time-dependent elements are independent of the initial values of the system.

  14. Activity-composition relations in the system CaCO 3-MgCO 3 predicted from static structure energy calculations and Monte Carlo simulations

    NASA Astrophysics Data System (ADS)

    Vinograd, Victor L.; Burton, Benjamin P.; Gale, Julian D.; Allan, Neil L.; Winkler, Björn

    2007-02-01

    Thermodynamic mixing properties and subsolidus phase relations of the rhombohedral carbonate system, (1 - x) · CaCO 3 - x · MgCO 3, were modelled in the temperature range of 623-2023 K with static structure energy calculations based on well-parameterised empirical interatomic potentials. Relaxed static structure energies of a large set of randomly varied structures in a 4 × 4 × 1 supercell of R3¯c calcite ( a = 19.952 Å, c = 17.061 Å) were calculated with the General Utility Lattice Program (GULP). These energies were cluster expanded in a basis set of 12 pair-wise effective interactions. Temperature-dependent enthalpies of mixing were calculated by the Monte Carlo method. Free energies of mixing were obtained by thermodynamic integration of the Monte Carlo results. The calculated phase diagram is in good agreement with experimental phase boundaries.

  15. [Determination of natural radioactive nuclides in the travertine samples from Tamagawa hot spring].

    PubMed

    Hashimoto, T; Masumura, S; Takahashi, K; Sotobayashi, T

    1982-07-01

    The determination of natural radioactive nuclides was carried out for 7 travertine samples collected from Tamagawa hot spring by means of the non-distructive gamma-ray spectrometry and of the alpha-ray spectrometry. From the former measurements, the relative activity strength, due to 223Ra, 226Ra, and 228Th, and their ratios was obtained in comparison with the photopeak strength due to respective daughters, 228Ac, 214Bi, and 212Pb, and with the results from a monazite sand standard. One travertine sample was engaged to the alpha-ray spectrometric determination of Th isotopes after the chemical purification using a 234Th-yield tracer. On the basis of the resultant absolute content of 228Th, the 228Ra and 228Th contents in the remainder samples were evaluated to be the range of 3 approximately 80 Bq (81 approximately 2160 pCi)/g and 2 approximately 20 Bq (54 approximately pCi)/g respectively. These radioactive nuclides were verified to exist almost within a Hokutolite small crystals up to 90% and there are apparently the radioactive disequilibrium relations between 228Ra and 228Th among freshly deposited travertines. The presence of 227Ac in Hokutolite was also suggested from the detection of 227Th owing to 215Po-alpha peak. PMID:7178540

  16. Runoff and sediment yield model for predicting nuclide transport in watersheds using BIOTRAN

    SciTech Connect

    Gallegos, A.F.; Wenzel, W.J.

    1990-09-01

    The environmental risk simulation model BIOTRAN was interfaced with a series of new subroutines (RUNOFF, GEOFLX, EROSON, and AQUIFER) to predict the movement of nuclides, elements, and pertinent chemical compounds in association with sediments through lateral and channel flow of runoff water. In addition, the movement of water into and out of segmented portions of runoff channels was modeled to simulate the dynamics of moisture flow through specified aquifers within the watershed. The BIOTRAN soil water flux subroutine, WATFLX, was modified to interface the relationships found in the SPUR model for runoff and sediment transport into channels with the particle sorting relationships to predict radionuclide enrichment and movement in watersheds. The new subroutines were applied specifically to Mortandad Canyon within Los Alamos National Laboratory by simultaneous simulation of eight surface vegetational subdivisions and associated channel and aquifer segments of this watershed. This report focuses on descriptions of the construction and rationale for the new subroutines and on discussing both input characteristics and output relationships to known runoff events from Mortandad Canyon. Limitations of the simplified input on model behavior are also discussed. Uranium-238 was selected as the nuclide for demonstration of the model because it could be assumed to be homogeneously distributed over the watershed surface. 22 refs., 18 figs., 9 tabs.

  17. Progress on multi-nuclide AMS of JAEA-AMS-TONO

    NASA Astrophysics Data System (ADS)

    Saito-Kokubu, Yoko; Matsubara, Akihiro; Miyake, Masayasu; Nishizawa, Akimitsu; Ohwaki, Yoshio; Nishio, Tomohiro; Sanada, Katsuki; Hanaki, Tatsumi

    2015-10-01

    The JAEA-AMS-TONO (Japan Atomic Energy Agency's Accelerator Mass Spectrometer established at the Tono Geoscience Center) facility has been used for the dating of geological samples. The AMS system is versatile, based on a 5 MV tandem Pelletron-type accelerator. Since its establishment in 1997, the AMS system has been used for measurement of carbon-14 (14C) mainly for 14C dating studies in neotectonics and hydrogeology, in support of JAEA's research on geosphere stability applicable to the long-term isolation of high-level radioactive waste. Results of the measurement of 14C in soils and plants has been applied to the dating of fault activity and volcanism. Development of beryllium-10 (10Be) and aluminum-26 (26Al) AMS systems are now underway to enhance the capability of the multi-nuclide AMS in studies of dating by cosmogenic nuclides. The 10Be-AMS system has already been used for routine measurements in applied studies and improvements of the measurement technique have been made. Now we plan to fine tune the system and perform test measurements to develop the 26Al-AMS system.

  18. Comparative studies in direct slow-neutron capture calculations

    SciTech Connect

    Mughabghab, S.F.

    1987-08-01

    Primary E1 transitions due to thermal neutron capture by the nuclides /sup 9/Be, /sup 32,34/S, /sup 40,42,44,46,48/Ca, and /sup 58/Ni are quantitatively interpreted by the Lane-Lynn formula and are compared with recent optical model calculations. The two approaches are equivalent provided the internal region of the nucleus is excluded in the optical model approach. Theoretical justifications for such a procedure are briefly presented. 32 refs., 4 tabs.

  19. Detailed Burnup Calculations for Testing Nuclear Data

    NASA Astrophysics Data System (ADS)

    Leszczynski, F.

    2005-05-01

    A general method (MCQ) has been developed by introducing a microscopic burnup scheme that uses the Monte Carlo calculated fluxes and microscopic reaction rates of a complex system and a depletion code for burnup calculations as a basis for solving nuclide material balance equations for each spatial region in which the system is divided. Continuous energy-dependent cross-section libraries and full 3D geometry of the system can be input for the calculations. The resulting predictions for the system at successive burnup time steps are thus based on a calculation route where both geometry and cross sections are accurately represented, without geometry simplifications and with continuous energy data, providing an independent approach for benchmarking other methods and nuclear data of actinides, fission products, and other burnable absorbers. The main advantage of this method over the classical deterministic methods currently used is that the MCQ System is a direct 3D method without the limitations and errors introduced on the homogenization of geometry and condensation of energy of deterministic methods. The Monte Carlo and burnup codes adopted until now are the widely used MCNP and ORIGEN codes, but other codes can be used also. For using this method, there is need of a well-known set of nuclear data for isotopes involved in burnup chains, including burnable poisons, fission products, and actinides. For fixing the data to be included in this set, a study of the present status of nuclear data is performed, as part of the development of the MCQ method. This study begins with a review of the available cross-section data of isotopes involved in burnup chains for power and research nuclear reactors. The main data needs for burnup calculations are neutron cross sections, decay constants, branching ratios, fission energy, and yields. The present work includes results of selected experimental benchmarks and conclusions about the sensitivity of different sets of cross

  20. Apparatus and method for quantitatively evaluating total fissile and total fertile nuclide content in samples. [Patent application

    DOEpatents

    Caldwell, J.T.; Kunz, W.E.; Cates, M.R.; Franks, L.A.

    1982-07-07

    Simultaneous photon and neutron interrogation of samples for the quantitative determination of total fissile nuclide and total fertile nuclide material present is made possible by the use of an electron accelerator. Prompt and delayed neutrons produced from resulting induced fission are counted using a single detection system and allow the resolution of the contributions from each interrogating flux leading in turn to the quantitative determination sought. Detection limits for /sup 239/Pu are estimated to be about 3 mg using prompt fission neutrons and about 6 mg using delayed neutrons.

  1. Code System to Calculate Mixed Cores in TRIGA Mark II Research Reactor.

    Energy Science and Technology Software Center (ESTSC)

    2001-08-29

    Version 00 TRIGLAV is a computer program for reactor calculations of mixed cores in a TRIGA Mark II research reactor. It can be applied for fuel element burn-up calculations, for power and flux distributions calculations and for reactivity predictions. The TRIGLAV program requires the WIMS-D4 program with the original WIMS cross-section library extended for TRIGA reactor specific nuclides. This package includes the code TRIGAC, which is a new version of TRIGAP.

  2. Extended scaling factors for in situ cosmogenic nuclides: New measurements at low latitude

    NASA Astrophysics Data System (ADS)

    Desilets, Darin; Zreda, Marek; Prabu, T.

    2006-06-01

    Production rates of cosmogenic nuclides at the earth's surface are controlled by the intensity of energetic cosmic-ray nucleons, which changes rapidly with elevation. An incomplete knowledge of how nucleon fluxes vary with elevation remains a major obstacle to utilizing cosmogenic nuclides as geochronometers in applications requiring highly accurate ages. One problem is that attenuation characteristics depend on nucleon energy. Measurements of high-energy (> 50 MeV) nucleon fluxes tend to give shorter attenuation lengths than low-energy (< 1 MeV) fluxes, but these differences are not well characterized due to a lack of data at lower energies. Another problem is that the atmospheric attenuation length for nucleon fluxes varies with the geomagnetic cutoff rigidity (a parameter related to geomagnetic latitude), RC, and that there has been an incomplete mapping of nucleon fluxes at high RC (low geomagnetic latitude). We report new measurements of nucleon fluxes from altitude transects in Hawaii ( RC = 12.8 GV) and Bangalore, India ( RC = 17.3 GV). Our measurements in Hawaii of low-energy neutrons (median energy 1 eV) and energetic nucleons (median energy 140 MeV) confirm that nucleon scaling functions are energy-dependent in the range of energies at which cosmogenic nuclides are produced. Our measurements in southern India extend our previously reported scaling model for spallation reactions [D. Desilets, M. Zreda, Spatial and temporal distribution of secondary cosmic-ray nucleon intensity and applications to in situ cosmogenic dating. Earth Planet. Sci. Lett. 206 (2003) 21-42] from RC = 13.3 GV to RC = 17.3 GV, nearly the highest cutoff rigidity on earth. The anomalously high cutoff rigidity over India provides a geomagnetic shielding condition that is effectively the same as would be observed at the geomagnetic equator in a dipole field with an intensity 1.2 times the modern value. This makes it possible to scale low-latitude production rates to paleomagnetic fields

  3. Implications of two Holocene time-dependent geomagnetic models for cosmogenic nuclide production rate scaling

    NASA Astrophysics Data System (ADS)

    Lifton, Nathaniel

    2016-01-01

    The geomagnetic field is a major influence on in situ cosmogenic nuclide production rates at a given location (in addition to atmospheric pressure and, to a lesser extent, solar modulation effects). A better understanding of how past fluctuations in these influences affected production rates should allow more accurate application of cosmogenic nuclides. As such, this work explores the cosmogenic nuclide production rate scaling implications of two recent time-dependent spherical harmonic geomagnetic models spanning the Holocene. Korte and Constable (2011, Phys. Earth Planet. Inter.188, 247-259) and Korte et al. (2011, Earth Planet. Sci. Lett. 312, 497-505) recently updated earlier spherical harmonic paleomagnetic models with new paleomagnetic data from sediment cores in addition to new archeomagnetic and volcanic data. These updated models offer improved resolution and accuracy over the previous versions, in part due to increased temporal and spatial data coverage. In addition, Pavón-Carrasco et al. (2014, Earth Planet. Sci. Lett. 388, 98-109) developed another time-dependent spherical harmonic model of the Holocene geomagnetic field, based solely on archeomagnetic and volcanic paleomagnetic data from the same underlying paleomagnetic database as the Korte et al. models, but extending to 14 ka. With the new models as input, trajectory-traced estimates of effective vertical cutoff rigidity (RC - the standard method for ordering cosmic ray data) yield significantly different time-integrated scaling predictions when compared to each other and to results using the earlier models. In addition, predictions of each new model using RC are tested empirically using recently published production rate calibration data for both 10Be and 3He, and compared to predictions using corresponding time-varying geocentric dipolar RC formulations and a static geocentric axial dipole (GAD) model. Results for the few calibration sites from geomagnetically sensitive regions suggest that the

  4. Comparing Time-Dependent Geomagnetic and Atmospheric Effects on Cosmogenic Nuclide Production Rate Scaling

    NASA Astrophysics Data System (ADS)

    Lifton, N. A.

    2014-12-01

    A recently published cosmogenic nuclide production rate scaling model based on analytical fits to Monte Carlo simulations of atmospheric cosmic ray flux spectra (both of which agree well with measured spectra) (Lifton et al., 2014, Earth Planet. Sci. Lett. 386, 149-160: termed the LSD model) provides two main advantages over previous scaling models: identification and quantification of potential sources of bias in the earlier models, and the ability to generate nuclide-specific scaling factors easily for a wide range of input parameters. The new model also provides a flexible framework for exploring the implications of advances in model inputs. In this work, the scaling implications of two recent time-dependent spherical harmonic geomagnetic models spanning the Holocene will be explored. Korte and Constable (2011, Phys. Earth Planet. Int. 188, 247-259) and Korte et al. (2011, Earth Planet. Sci. Lett. 312, 497-505) recently updated earlier spherical harmonic paleomagnetic models used by Lifton et al. (2014) with paleomagnetic measurements from sediment cores in addition to archeomagnetic and volcanic data. These updated models offer improved accuracy over the previous versions, in part to due to increased temporal and spatial data coverage. With the new models as input, trajectory-traced estimates of effective vertical cutoff rigidity (RC- the standard method for ordering cosmic ray data) yield significantly different time-integrated scaling predictions when compared to the earlier models. These results will be compared to scaling predictions using another recent time-dependent spherical harmonic model of the Holocene geomagnetic field by Pavón-Carrasco et al. (2014, Earth Planet. Sci. Lett. 388, 98-109), based solely on archeomagnetic and volcanic paleomagnetic data, but extending to 14 ka. In addition, the potential effects of time-dependent atmospheric models on LSD scaling predictions will be presented. Given the typical dominance of altitudinal over

  5. Regional Dispersal of Fukushima-derived Fission Nuclides by East Asia Monsoon

    NASA Astrophysics Data System (ADS)

    Huh, Chih-An; Lin, Chuan-Yao; Hsu, Shih-Chieh

    2013-04-01

    Since the Fukushima nuclear accident happened on 12 March 2011, there have been a plethora of publications about the dispersion of radioactive material from the damaged reactors. Most of these works dealt with global transport of Fukushima-derived radionuclides in the northern hemisphere and local transport in the vicinity of Fukushima and around Japan. In contrast, few works investigated into dispersal of radiation plumes from Japan to other areas on regional scales. This is because regional dispersal out of Japan in the springtime is most likely dominated by the northeastern monsoon, whereas there are few monitoring stations downwind in the southeastern Asia region. In this respect, we are only aware of the data in Vietnam published by Long et al (2012) in addition to our own data obtained in and around Taiwan (Huh et al., 2012; Hsu et al., 2012). By integrating the data published in the literature plus those that can be searched from relevant websites, we try to further elucidate the dispersal of Fukushima-derived radiation toward the southeastern Asia region. The WRF/Chem tracer model is employed to simulate the dispersal of radiation plumes from the damaged Fukushima Daiichi Nuclear Power Plant. From a vis-à-vis comparison between the model simulation and the time-series of Fukushima-derived fission nuclides monitored around the southeastern Asia, we can distinguish between global transport by the Westerlies in the free troposphere and regional transport by the northeast monsoon in the planetary boundary layer. In general, regional (mainly meridional) transport carried more weight than global (mainly zonal) transport in contributing Fukushima-derived radioactivity to the area covered in this review, particularly at the ground-level sites. References 1. Hsu, S.C., Huh, C.A., Chan, C.Y., Lin, S.H., Lin, F.J. and Liu, S.C. (2012). Hemispheric dispersion of radioactive plume laced with fission nuclides from the Fukushima nuclear event. Geophys. Res. Lett. 39, L00

  6. A counter-intuitive approach to calculating non-exchangeable 2H isotopic composition of hair: treating the molar exchange fraction fE as a process-related rather than compound-specific variable

    USGS Publications Warehouse

    Landwehr, J.M.; Meier-Augenstein, W.; Kemp, H.F.

    2011-01-01

    Hair is a keratinous tissue that incorporates hydrogen from material that an animal consumes but it is metabolically inert following synthesis. The stable hydrogen isotope composition of hair has been used in ecological studies to track migrations of mammals as well as for forensic and archaeological purposes to determine the provenance of human remains or the recent geographic life trajectory of living people. Measurement of the total hydrogen isotopic composition of a hair sample yields a composite value comprised of both metabolically informative, non-exchangeable hydrogen and exchangeable hydrogen, with the latter reflecting ambient or sample preparation conditions. Neither of these attributes is directly measurable, and the non-exchangeable hydrogen composition is obtained by estimation using a commonly applied mathematical expression incorporating sample measurements obtained from two distinct equilibration procedures. This commonly used approach treats the fraction of exchangeable hydrogen as a mixing ratio, with a minimal procedural fractionation factor assumed to be close or equal to 1. Instead, we propose to use full molar ratios to derive an expression for the non-exchangeable hydrogen composition explicitly as a function of both the procedural fractionation factor α and the molar hydrogen exchange fraction fE. We apply these derivations in a longitudinal study of a hair sample and demonstrate that the molar hydrogen exchange fraction fE should, like the procedural fractionation factor α, be treated as a process-dependent parameter, i.e. a reaction-specific constant. This is a counter-intuitive notion given that maximum theoretical values for the molar hydrogen exchange fraction fE can be calculated that are arguably protein-type specific and, as such, fE could be regarded as a compound-specific constant. We also make some additional suggestions for future approaches to determine the non-exchangeable hydrogen composition of hair and the use of

  7. Towards a magnetic field stabilization at ISOLTRAP for high-accuracy mass measurements on exotic nuclides

    NASA Astrophysics Data System (ADS)

    Marie-Jeanne, M.; Alonso, J.; Blaum, K.; Djekic, S.; Dworschak, M.; Hager, U.; Herlert, A.; Nagy, Sz.; Savreux, R.; Schweikhard, L.; Stahl, S.; Yazidjian, C.

    2008-03-01

    The field stability of a mass spectrometer plays a crucial role in the accuracy of mass measurements. In the case of mass determination of short-lived nuclides with a Penning trap, major causes of fluctuations are temperature variations in the vicinity of the trap and pressure changes in the liquid helium cryostat of the superconducting magnet. Thus systems for the temperature and pressure stabilization of the Penning trap mass spectrometer ISOLTRAP at the ISOLDE facility at CERN have been installed. A reduction of the temperature and pressure fluctuations by at least an order of magnitude down to ΔT≈±5 mK and Δp≈±5 Pa has been achieved, which corresponds to a relative magnetic field change of ΔB/B=2.7×10-9 and 1.1×10-10, respectively.

  8. Atomic mass measurements of short-lived nuclides around the doubly-magic 208Pb

    NASA Astrophysics Data System (ADS)

    Weber, C.; Audi, G.; Beck, D.; Blaum, K.; Bollen, G.; Herfurth, F.; Kellerbauer, A.; Kluge, H.-J.; Lunney, D.; Schwarz, S.

    2008-04-01

    Accurate atomic mass measurements of neutron-deficient and neutron-rich nuclides around the doubly-magic 208Pb and of neutron-rich cesium isotopes were performed with the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The masses of 145,147Cs, 181,183Tl, 186Tl m, 187Tl m, 196Tl m, 205Tl, 197Pb m, 208Pb, 190-197Bi, 209,215,216Bi, 203,205,229Fr, and 214,229,230Ra were determined. The obtained relative mass uncertainty in the range of 2×10 to 2×10 is not only required for safe identification of isomeric states but also allows mapping the detailed structure of the mass surface. A mass adjustment procedure was carried out and the results included into the Atomic Mass Evaluation. The resulting separation energies are discussed and the mass spectrometric and laser spectroscopic data are examined for possible correlations.

  9. Vapor pressures and calculated heats of vaporization of concentrated nitric acid solutions in the composition range 71 to 89 percent nitrogen dioxide, 1 to 10 percent water, and in the temperature range 10 to 60 degrees C

    NASA Technical Reports Server (NTRS)

    Mckeown, A B; Belles, Frank E

    1954-01-01

    Total vapor pressures were measured for 16 acid mixtures of the ternary system nitric acid, nitrogen dioxide, and water within the temperature range 10 degrees to 60 degrees Celsius, and with the composition range 71 to 89 weight percent nitric acid, 7 to 20 weight percent nitrogen dioxide, and 1 to 10 weight percent water. Heats of vaporization were calculated from the vapor pressure measurements for each sample for the temperatures 25, 40, and 60 degrees Celsius. The ullage of the apparatus used for the measurements was 0.46. Ternary diagrams showing isobars as a function of composition of the system were constructed from experimental and interpolated data for the temperatures 25, 40, 45, and 60 degrees C and are presented herein.

  10. Probing the nuclides {sup 102}Pd, {sup 106}Cd, and {sup 144}Sm for resonant neutrinoless double-electron capture

    SciTech Connect

    Goncharov, M.; Blaum, K.; Eliseev, S.; Block, M.; Herfurth, F.; Minaya Ramirez, E.; Droese, C.; Schweikhard, L.; Novikov, Yu. N.; Zuber, K.

    2011-08-15

    The Q values for double-electron capture in {sup 102}Pd, {sup 106}Cd, and {sup 144}Sm have been measured by Penning-trap mass spectrometry. The results exclude at present all three nuclides from the list of suitable candidates for a search for resonant neutrinoless double-electron capture.