Tobin, J G; Yu, S W; Komesu, T; Chung, B W; Morton, S A; Waddill, G D
2006-03-31
Using Fano Effect measurements upon polycrystalline Ce, we have observed a phase reversal between the spectral structure at the Fermi Edge and the other 4f derived feature near a binding energy of 2 eV. The Fano Effect is the observation of spin polarized photoelectron emission from NONMAGNETIC materials, under chirally selective excitation, such as circularly polarized photons. Within various models, the peak at the Fermi Energy (f{sup 1} peak, quasiparticle peak, Kondo peak) is predicted to be the manifestation of the electrons which shield the otherwise unpaired spin associated with the peak at 2 eV (f{sup 0} peak or Lower Hubbard Band). Utilizing high-energy photoelectron spectroscopy, on and off resonance, the bulk nature and f-character of both features have been confirmed. Thus, observation of phase reversal between the f{sup 0} and f{sup 1} peak is a direct experimental proof of spin shielding in Ce, confirming the original model of Gunnarsson and Shoenhammer, albeit within a Hubbard picture.
Dynamic rotating-shield brachytherapy
Liu, Yunlong; Flynn, Ryan T.; Kim, Yusung; Yang, Wenjun; Wu, Xiaodong
2013-12-15
Purpose: To present dynamic rotating shield brachytherapy (D-RSBT), a novel form of high-dose-rate brachytherapy (HDR-BT) with electronic brachytherapy source, where the radiation shield is capable of changing emission angles during the radiation delivery process.Methods: A D-RSBT system uses two layers of independently rotating tungsten alloy shields, each with a 180° azimuthal emission angle. The D-RSBT planning is separated into two stages: anchor plan optimization and optimal sequencing. In the anchor plan optimization, anchor plans are generated by maximizing the D{sub 90} for the high-risk clinical-tumor-volume (HR-CTV) assuming a fixed azimuthal emission angle of 11.25°. In the optimal sequencing, treatment plans that most closely approximate the anchor plans under the delivery-time constraint will be efficiently computed. Treatment plans for five cervical cancer patients were generated for D-RSBT, single-shield RSBT (S-RSBT), and {sup 192}Ir-based intracavitary brachytherapy with supplementary interstitial brachytherapy (IS + ICBT) assuming five treatment fractions. External beam radiotherapy doses of 45 Gy in 25 fractions of 1.8 Gy each were accounted for. The high-risk clinical target volume (HR-CTV) doses were escalated such that the D{sub 2cc} of the rectum, sigmoid colon, or bladder reached its tolerance equivalent dose in 2 Gy fractions (EQD2 with α/β= 3 Gy) of 75 Gy, 75 Gy, or 90 Gy, respectively.Results: For the patients considered, IS + ICBT had an average total dwell time of 5.7 minutes/fraction (min/fx) assuming a 10 Ci{sup 192}Ir source, and the average HR-CTV D{sub 90} was 78.9 Gy. In order to match the HR-CTV D{sub 90} of IS + ICBT, D-RSBT required an average of 10.1 min/fx more delivery time, and S-RSBT required 6.7 min/fx more. If an additional 20 min/fx of delivery time is allowed beyond that of the IS + ICBT case, D-RSBT and S-RSBT increased the HR-CTV D{sub 90} above IS + ICBT by an average of 16.3 Gy and 9.1 Gy, respectively
Brodsky, Stanley J.
2002-01-09
Spin effects in exclusive and inclusive reactions provide an essential new dimension for testing QCD and unraveling hadron structure. Remarkable new experiments from SLAC, HERMES (DESY), and Jefferson Lab present many challenges to theory, including measurements at HERMES and SMC of the single spin asymmetries in ep {yields} e{prime}{pi}X where the proton is polarized normal to the scattering plane. This type of single spin asymmetry may be due to the effects of rescattering of the outgoing quark on the spectators of the target proton, an effect usually neglected in conventional QCD analyses. Many aspects of spin, such as single-spin asymmetries and baryon magnetic moments are sensitive to the dynamics of hadrons at the amplitude level, rather than probability distributions. I will illustrate the novel features of spin dynamics for relativistic systems by examining the explicit form of the light-front wavefunctions for the two-particle Fock state of the electron in QED, thus connecting the Schwinger anomalous magnetic moment to the spin and orbital momentum carried by its Fock state constituents and providing a transparent basis for understanding the structure of relativistic composite systems and their matrix elements in hadronic physics. I also present a survey of outstanding spin puzzles in QCD, particularly A{sub NN} in elastic pp scattering, the J/{psi} {yields} {rho}{pi} puzzle, and J/{psi} polarization at the Tevatron.
Ning, F. L.; Ahilan, K.; Imai, T.; Sefat, A. S.; McGuire, Michael A; Sales, Brian C; Mandrus, David; Cheng, P.; Shen, B.; Wen, H.-H.
2010-01-01
We report the first NMR investigation of spin dynamics in the overdoped nonsuperconducting regime of Ba(Fe{sub 1-x}Co{sub x}){sub 2}As{sub 2} up to x=0.26. We demonstrate that the absence of interband transitions with large momentum transfer Q{sub AF}-({pi}/a,0) between the hole and electron Fermi surfaces results in complete suppression of antiferromagnetic spin fluctuations for x {ge} 0.15. Our experimental results provide direct evidence for a correlation between T{sub c} and the strength of Q{sub AF} antiferromagnetic spin fluctuations.
Spin-rotation and NMR shielding constants in HCl
Jaszuński, Michał; Repisky, Michal; Demissie, Taye B.; Komorovsky, Stanislav; Malkin, Elena; Ruud, Kenneth; Garbacz, Piotr; Jackowski, Karol; Makulski, Włodzimierz
2013-12-21
The spin-rotation and nuclear magnetic shielding constants are analysed for both nuclei in the HCl molecule. Nonrelativistic ab initio calculations at the CCSD(T) level of approximation show that it is essential to include relativistic effects to obtain spin-rotation constants consistent with accurate experimental data. Our best estimates for the spin-rotation constants of {sup 1}H{sup 35}Cl are C{sub Cl} = −53.914 kHz and C{sub H} = 42.672 kHz (for the lowest rovibrational level). For the chlorine shielding constant, the ab initio value computed including the relativistic corrections, σ(Cl) = 976.202 ppm, provides a new absolute shielding scale; for hydrogen we find σ(H) = 31.403 ppm (both at 300 K). Combining the theoretical results with our new gas-phase NMR experimental data allows us to improve the accuracy of the magnetic dipole moments of both chlorine isotopes. For the hydrogen shielding constant, including relativistic effects yields better agreement between experimental and computed values.
Dynamical Analysis of the SHIELD Galaxies
NASA Astrophysics Data System (ADS)
McNichols, Andrew Thomas; Teich, Yaron G.; Cannon, John M.
2015-08-01
We present a dynamical analysis of the 12 extremely low-mass dwarf galaxies that comprise SHIELD, a product of the Arecibo Legacy Fast ALFA survey (ALFALFA). We use multi-configuration, high spatial (˜ 150 - 350 pc) and spectral (0.82 - 2.46 km s-1 ch-1) resolution data obtained from 21 cm observations conducted with the Karl G. Jansky Very Large Array. For each source, we attempt to derive an inclination-corrected rotation curve, to calculate the maximum rotation velocity (≤ 30 km s-1 for the survey population), and to further constrain the H I mass. For sources from which a sufficiently precise rotation curve can be derived, we use spatially resolved Spitzer Space Telescope 3.6 and 4.5 μm images to determine the stellar mass as a function of radius. The gaseous and stellar mass estimates are then used to decompose the total dynamical mass values and to obtain neutral gas fractions and relative baryonic content. Characterizing the kinematics of the SHIELD galaxies allows us to draw more general conclusions about the structure and dynamical evolution of low mass dwarf galaxies in the local universe.This work is a result of collaboration with the SHIELD Team and is supported by NSF grant 1211683.
SHIELD: Neutral Gas Kinematics and Dynamics
NASA Astrophysics Data System (ADS)
McNichols, Andrew; Teich, Yaron; Cannon, John M.; SHIELD Team
2016-01-01
The "Survey of HI in Extremely Low-mass Dwarfs" (SHIELD) is a multiwavelength, legacy-class observational study of 12 low-mass dwarf galaxies discovered in Arecibo Legacy Fast ALFA (ALFALFA) survey data products. Here we present new results of detailed kinematic analyses of these systems using multi-configuration, high spatial (˜300 pc) and spectral (0.82 - 2.46 km s-1 ch-1) resolution HI observations from the Karl G. Jansky Very Large Array. For each source, we produce velocity fields and dispersion maps using different spatial and spectral resolution representations of the data in order to attempt derivation of an inclination-corrected rotation curve. While both two- and three-dimensional fitting techniques are employed, the comparable magnitudes of velocity dispersion and projected rotation result in degeneracies that prohibit unambiguous circular velocity solutions. We thus make multiple position-velocity cuts across each galaxy to determine the maximum circular rotation velocity (≤ 30 km-1 for the survey population). Baryonic masses are calculated using single-dish H I fluxes from Arecibo and stellar masses derived from HST and Spitzer imaging. Comparison is made with total dynamical masses estimated from the position-velocity analysis. The SHIELD galaxies are contextualized on the baryonic Tully-Fisher relation.Support for this work was provided by NSF grant AST-1211683 to JMC at Macalester College.
Dynamic scaling in spin glasses
NASA Astrophysics Data System (ADS)
Pappas, C.; Mezei, F.; Ehlers, G.; Manuel, P.; Campbell, I. A.
2003-08-01
We present neutron spin echo (NSE) results and a revisited analysis of historical data on spin glasses, which reveal a pure power-law time decay of the spin autocorrelation function s(Q,t)=S(Q,t)/S(Q) at the glass temperature Tg. The power law exponent is in excellent agreement with that calculated from dynamic and static critical exponents deduced from macroscopic susceptibility measurements made on a quite different time scale. This scaling relation involving exponents of different physical quantities determined by completely independent experimental methods is stringently verified experimentally in a spin glass. As spin glasses are a subgroup of the vast family of glassy systems also comprising structural glasses and other noncrystalline systems the observed strict critical scaling behavior is important. Above the phase transition the strikingly nonexponential relaxation, best fitted by the Ogielski (power-law times stretched exponential) function, appears as an intrinsic, homogeneous feature of spin glasses.
Spin-current emission governed by nonlinear spin dynamics
Tashiro, Takaharu; Matsuura, Saki; Nomura, Akiyo; Watanabe, Shun; Kang, Keehoon; Sirringhaus, Henning; Ando, Kazuya
2015-01-01
Coupling between conduction electrons and localized magnetization is responsible for a variety of phenomena in spintronic devices. This coupling enables to generate spin currents from dynamical magnetization. Due to the nonlinearity of magnetization dynamics, the spin-current emission through the dynamical spin-exchange coupling offers a route for nonlinear generation of spin currents. Here, we demonstrate spin-current emission governed by nonlinear magnetization dynamics in a metal/magnetic insulator bilayer. The spin-current emission from the magnetic insulator is probed by the inverse spin Hall effect, which demonstrates nontrivial temperature and excitation power dependences of the voltage generation. The experimental results reveal that nonlinear magnetization dynamics and enhanced spin-current emission due to magnon scatterings are triggered by decreasing temperature. This result illustrates the crucial role of the nonlinear magnon interactions in the spin-current emission driven by dynamical magnetization, or nonequilibrium magnons, from magnetic insulators. PMID:26472712
Spin-current emission governed by nonlinear spin dynamics.
Tashiro, Takaharu; Matsuura, Saki; Nomura, Akiyo; Watanabe, Shun; Kang, Keehoon; Sirringhaus, Henning; Ando, Kazuya
2015-01-01
Coupling between conduction electrons and localized magnetization is responsible for a variety of phenomena in spintronic devices. This coupling enables to generate spin currents from dynamical magnetization. Due to the nonlinearity of magnetization dynamics, the spin-current emission through the dynamical spin-exchange coupling offers a route for nonlinear generation of spin currents. Here, we demonstrate spin-current emission governed by nonlinear magnetization dynamics in a metal/magnetic insulator bilayer. The spin-current emission from the magnetic insulator is probed by the inverse spin Hall effect, which demonstrates nontrivial temperature and excitation power dependences of the voltage generation. The experimental results reveal that nonlinear magnetization dynamics and enhanced spin-current emission due to magnon scatterings are triggered by decreasing temperature. This result illustrates the crucial role of the nonlinear magnon interactions in the spin-current emission driven by dynamical magnetization, or nonequilibrium magnons, from magnetic insulators. PMID:26472712
Electron spin decoherence in nuclear spin baths and dynamical decoupling
Zhao, N.; Yang, W.; Ho, S. W.; Hu, J. L.; Wan, J. T. K.; Liu, R. B.
2011-12-23
We introduce the quantum theory of the electron spin decoherence in a nuclear spin bath and the dynamical decoupling approach for protecting the electron spin coherence. These theories are applied to various solid-state systems, such as radical spins in molecular crystals and NV centers in diamond.
Measurements of nuclear spin dynamics by spin-noise spectroscopy
Ryzhov, I. I.; Poltavtsev, S. V.; Kozlov, G. G.; Zapasskii, V. S.; Kavokin, K. V.; Glazov, M. M.; Vladimirova, M.; Scalbert, D.; Cronenberger, S.; Lemaître, A.; Bloch, J.
2015-06-15
We exploit the potential of the spin noise spectroscopy (SNS) for studies of nuclear spin dynamics in n-GaAs. The SNS experiments were performed on bulk n-type GaAs layers embedded into a high-finesse microcavity at negative detuning. In our experiments, nuclear spin polarisation initially prepared by optical pumping is monitored in real time via a shift of the peak position in the electron spin noise spectrum. We demonstrate that this shift is a direct measure of the Overhauser field acting on the electron spin. The dynamics of nuclear spin is shown to be strongly dependent on the electron concentration.
Microscopic studies of nonlocal spin dynamics and spin transport (invited)
Adur, Rohan; Du, Chunhui; Cardellino, Jeremy; Scozzaro, Nicolas; Wolfe, Christopher S.; Wang, Hailong; Herman, Michael; Bhallamudi, Vidya P.; Pelekhov, Denis V.; Yang, Fengyuan; Hammel, P. Chris
2015-05-07
Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.
Microscopic studies of nonlocal spin dynamics and spin transport (invited)
NASA Astrophysics Data System (ADS)
Adur, Rohan; Du, Chunhui; Cardellino, Jeremy; Scozzaro, Nicolas; Wolfe, Christopher S.; Wang, Hailong; Herman, Michael; Bhallamudi, Vidya P.; Pelekhov, Denis V.; Yang, Fengyuan; Hammel, P. Chris
2015-05-01
Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.
Spin dynamics simulations at AGS
Huang, H.; MacKay, W.W.; Meot, F.; Roser, T.
2010-05-23
To preserve proton polarization through acceleration, it is important to have a correct model of the process. It has been known that with the insertion of the two helical partial Siberian snakes in the Alternating Gradient Synchrotron (AGS), the MAD model of AGS can not deal with a field map with offset orbit. The stepwise ray-tracing code Zgoubi provides a tool to represent the real electromagnetic fields in the modeling of the optics and spin dynamics for the AGS. Numerical experiments of resonance crossing, including spin dynamics in presence of the snakes and Q-jump, have been performed in AGS lattice models, using Zgoubi. This contribution reports on various results so obtained.
Spin dynamics with inertia in metallic ferromagnets
NASA Astrophysics Data System (ADS)
Kikuchi, Toru; Tatara, Gen
2015-11-01
The nonadiabatic contribution of environmental degrees of freedom yields an effective inertia of spin in the effective spin dynamics. In this paper, we study several aspects of the inertia of spin in metallic ferromagnets: (i) a concrete expression of the spin inertia ms: ms=ℏ Sc/(2 gsd) , where Sc is the spin polarization of conduction electrons and gsd is the s d coupling constant; (ii) a dynamical behavior of spin with inertia, discussed from the viewpoints of a spinning top and of a particle on a sphere; (iii) the behavior of spin waves and domain walls in the presence of inertia and the behavior of spin with inertia under a time-dependent magnetic field.
Coherent spin mixing dynamics in a spin-1 atomic condensate
Zhang Wenxian; Chang, M.-S.; Chapman, M.S.; Zhou, D.L.; You, L.
2005-07-15
We study the coherent off-equilibrium spin mixing inside an atomic condensate. Using mean-field theory and adopting the single-spatial-mode approximation, the condensate spin dynamics is found to be well described by that of a nonrigid pendulum and displays a variety of periodic oscillations in an external magnetic field. Our results illuminate several recent experimental observations and provide critical insights into the observation of coherent interaction-driven oscillations in a spin-1 condensate.
NASA Astrophysics Data System (ADS)
Fideles, Bruna; Oliveira, Leonardo B. A.; Colherinhas, Guilherme
2016-01-01
We investigate the nuclear isotropic shielding constants and spin-spin coupling for oxygen and carbons atoms of isomers of tartaric acid in gas phase and in water solutions by Monte Carlo simulation and quantum mechanics calculations using the GIAO-B3LYP approach. Solute polarization effects are included iteratively and play an important role in the quantitative determination of shielding constants. Our MP2/aug-cc-pVTZ results show substantial increases of the dipole moment in solution as compared with the gas phase results (61-221%). The solvent effects on the σ(13O) values are in general small. More appreciable solvent effects can be seen on the σ(17O) and J(Csbnd O).
Electron-spin dynamics induced by photon spins
NASA Astrophysics Data System (ADS)
Bauke, Heiko; Ahrens, Sven; Keitel, Christoph H.; Grobe, Rainer
2014-10-01
Strong rotating magnetic fields may cause a precession of the electron's spin around the rotation axis of the magnetic field. The superposition of two counterpropagating laser beams with circular polarization and opposite helicity features such a rotating magnetic field component but also carries spin. The laser's spin density, which can be expressed in terms of the laser's electromagnetic fields and potentials, couples to the electron's spin via a relativistic correction to the Pauli equation. We show that the quantum mechanical interaction of the electron's spin with the laser's rotating magnetic field and with the laser's spin density counteract each other in such a way that a net spin rotation remains with a precession frequency that is much smaller than the frequency one would expect from the rotating magnetic field alone. In particular, the frequency scales differently with the laser's electric field strength depending on whether relativistic corrections are taken into account or not. Thus, the relativistic coupling of the electron's spin to the laser's spin density changes the dynamics not only quantitatively but also qualitatively as compared to the nonrelativistic theory. The electron's spin dynamics are a genuine quantum mechanical relativistic effect.
Electrically Driven Spin Dynamics of Paramagnetic Impurities
NASA Astrophysics Data System (ADS)
Saha, D.; Siddiqui, L.; Bhattacharya, P.; Datta, S.; Basu, D.; Holub, M.
2008-05-01
The spin dynamics of dilute paramagnetic impurities embedded in a semiconductor GaAs channel of a conventional lateral spin valve has been investigated. It is observed that the electron spin of paramagnetic Mn atoms can be polarized electrically when driven by a spin valve in the antiparallel configuration. The transient current through the MnAs/GaAs/MnAs spin valve bears the signature of the underlying spin dynamics driven by the exchange interaction between the conduction band electrons in GaAs and the localized Mn electron spins. The time constant for this interaction is observed to be dependent on temperature and is estimated to be 80 ns at 15 K.
Electrically driven spin dynamics of paramagnetic impurities.
Saha, D; Siddiqui, L; Bhattacharya, P; Datta, S; Basu, D; Holub, M
2008-05-16
The spin dynamics of dilute paramagnetic impurities embedded in a semiconductor GaAs channel of a conventional lateral spin valve has been investigated. It is observed that the electron spin of paramagnetic Mn atoms can be polarized electrically when driven by a spin valve in the antiparallel configuration. The transient current through the MnAs/GaAs/MnAs spin valve bears the signature of the underlying spin dynamics driven by the exchange interaction between the conduction band electrons in GaAs and the localized Mn electron spins. The time constant for this interaction is observed to be dependent on temperature and is estimated to be 80 ns at 15 K. PMID:18518470
Dynamics of antiferromagnets driven by spin current
NASA Astrophysics Data System (ADS)
Cheng, Ran; Niu, Qian
2014-02-01
When a spin-polarized current flows through a ferromagnetic (FM) metal, angular momentum is transferred to the background magnetization via spin-transfer torques. In antiferromagnetic (AFM) materials, however, the corresponding problem is unsolved. We derive microscopically the dynamics of an AFM system driven by spin current generated by an attached FM polarizer, and find that the spin current exerts a driving force on the local staggered order parameter. The mechanism does not rely on the conservation of spin angular momentum, nor does it depend on the induced FM moments on top the AFM background. Two examples are studied: (i) A domain wall is accelerated to a terminal velocity by purely adiabatic effect where the Walker's breakdown is avoided. (ii) Spin injection modifies the AFM resonance frequency, and spin current injection triggers spin wave instability of local moments above a threshold.
Spin dynamics in paramagnetic diluted magnetic semiconductors
NASA Astrophysics Data System (ADS)
Phan, Van-Nham; Tran, Minh-Tien
2015-10-01
Microscopic properties of low-energy spin dynamics in diluted magnetic semiconductor are addressed in a framework of the Kondo lattice model including random distribution of magnetic dopants. Based on the fluctuation-dissipation theorem, we derive an explicit dependence of the spin diffusion coefficient on the single-particle Green function which is directly evaluated by dynamical mean-field theory. In the paramagnetic state, the magnetic scattering has been manifested to suppress spin diffusion. In agreement with other ferromagnet systems, we also point out that the spin diffusion in diluted magnetic semiconductors at small carrier concentration displays a monotonic 1 /T -like temperature dependence. By investigating the spin diffusion coefficient on a wide range of the model parameters, the obtained results have provided a significant scenario to understand the spin dynamics in the paramagnetic diluted magnetic semiconductors.
Spin dynamics in driven composite multiferroics
Wang, Zidong Grimson, Malcolm J.
2015-09-28
A spin dynamics approach has been used to study the behavior of the magnetic spins and the electric pseudo-spins in a 1-D composite multiferroic chain with a linear magneto-electric coupling at the interface. The response is investigated with either external magnetic or electric fields driving the system. The spin dynamics is based on the Landau-Lifshitz-Gilbert equation. A Gaussian white noise is later added into the dynamic process to include the thermal effects. The interface requires a closer inspection of the magneto-electric effects. Thus, we construct a 2-D ladder model to describe the behavior of the magnetic spins and the electric pseudo-spins with different magneto-electric couplings.
Spin dynamics in driven composite multiferroics
NASA Astrophysics Data System (ADS)
Wang, Zidong; Grimson, Malcolm J.
2015-09-01
A spin dynamics approach has been used to study the behavior of the magnetic spins and the electric pseudo-spins in a 1-D composite multiferroic chain with a linear magneto-electric coupling at the interface. The response is investigated with either external magnetic or electric fields driving the system. The spin dynamics is based on the Landau-Lifshitz-Gilbert equation. A Gaussian white noise is later added into the dynamic process to include the thermal effects. The interface requires a closer inspection of the magneto-electric effects. Thus, we construct a 2-D ladder model to describe the behavior of the magnetic spins and the electric pseudo-spins with different magneto-electric couplings.
Exploring the quantum frontier of spin dynamics
NASA Astrophysics Data System (ADS)
Bruno, Patrick
2011-03-01
Our familiar classical concept of a spin is that of a system characterized by the direction in which the spin is pointing. In this picture, we may think of the dynamics of a spin as the motion of a classical gyroscope, wich we can aptly describe the spin dynamics as the motion of a point on a sphere. This classical description of the spin dynamics, formalized in the Landau-Lifshits-Gilbert equation, has proved extremely successful in the field micro- and nanomagnetism. However, as the size of the system is further decreased (e.g., when considering molecular magnets such as the Fe 8 or Mn 12 systems, which have a spin S = 10), quantum effects such as tunneling, interference, entanglement, coherence, etc., play an essential role, and one must adopt a fully quantum mechanical description of the spin system. The landscape in which the system evolves is then no longer a mere sphere, but rather it is the projective Hilbert space (wich is the projective complex space <= P2S for a spin S) , as space of considerably greater richness and complexity than the sphere of classical spin dynamics. A very appealing tool to describe a quantum spin system is Majorana's stellar representation, which is the extension for a spin S of the Bloch sphere description of a spin / 1 2 . I shall discuss how this representation can help us in improving our understanding of fundamental quantum processes and concept such as Landau-Zener transitions, Rabi oscillations, Berry phase, diabolical points and illustrate this on the example of spin dynamics of molecular magnets.
Seeing Spin Dynamics in Atomic Gases
NASA Astrophysics Data System (ADS)
Stamper-Kurn, Dan M.
2015-06-01
The dynamics of internal spin, electronic orbital, and nuclear motion states of atoms and molecules have preoccupied the atomic and molecular physics community for decades. Increasingly, such dynamics are being examined within many-body systems composed of atomic and molecular gases. Our findings sometimes bear close relation to phenomena observed in condensed-matter systems, while on other occasions they represent truly new areas of investigation. I discuss several examples of spin dynamics that occur within spinor Bose-Einstein gases, highlighting the advantages of spin-sensitive imaging for understanding and utilizing such dynamics.
Glassy Spin Dynamics in Buckled Colloidal Crystal
NASA Astrophysics Data System (ADS)
Zhou, Di; Wang, Feng; Han, Yilong
Geometric frustration arises when lattice structure prevents simultaneous minimization of local interaction energies. It leads to highly degenerate ground states and complex behaviors in frustrated magnetic materials. Here we experimentally studied buckled 1.5-layer colloidal NIPA microgel crystals confined between parallel plates. Spheres buckled up and down are analogous to antiferromagnetic Ising spins. These spins on the distorted triangular lattice exhibit glassy dynamics at low temperatures. In particular, a spin only has 13 nearest-neighbor configurations, which enables to reveal the correlation between structures and dynamical heterogeneity. Soft modes also localize at high-energy regions. Further, we compared the colloidal spin system with kinetic constrained models (KCMs) and observed dynamical facilitation behaviors including excitations lines in space-time. Similar structures and glassy dynamics are also observed in our simulation of Coulomb charges on a triangular lattice. The work was supported by Grant RGC-GRF601613.
Tang, Yanhao; Xie, Wei; McGuire, John A. Lai, Chih Wei; Mandal, Krishna C.
2015-09-21
We analyze exciton spin dynamics in GaSe under nonresonant circularly polarized optical pumping with an exciton spin-flip rate-equation model. The model reproduces polarized time-dependent photoluminescence measurements in which the initial circular polarization approaches unity even when pumping with 0.15 eV excess energy. At T = 10 K, the exciton spin relaxation exhibits a biexponential decay with sub-20 ps and >500 ps time constants, which are also reproduced by the rate-equation model assuming distinct spin-relaxation rates for hot (nonequilibrium) and cold band-edge excitons.
Ab initio non-relativistic spin dynamics
Ding, Feizhi; Goings, Joshua J.; Li, Xiaosong; Frisch, Michael J.
2014-12-07
Many magnetic materials do not conform to the (anti-)ferromagnetic paradigm where all electronic spins are aligned to a global magnetization axis. Unfortunately, most electronic structure methods cannot describe such materials with noncollinear electron spin on account of formally requiring spin alignment. To overcome this limitation, it is necessary to generalize electronic structure methods and allow each electron spin to rotate freely. Here, we report the development of an ab initio time-dependent non-relativistic two-component spinor (TDN2C), which is a generalization of the time-dependent Hartree-Fock equations. Propagating the TDN2C equations in the time domain allows for the first-principles description of spin dynamics. A numerical tool based on the Hirshfeld partitioning scheme is developed to analyze the time-dependent spin magnetization. In this work, we also introduce the coupling between electron spin and a homogenous magnetic field into the TDN2C framework to simulate the response of the electronic spin degrees of freedom to an external magnetic field. This is illustrated for several model systems, including the spin-frustrated Li{sub 3} molecule. Exact agreement is found between numerical and analytic results for Larmor precession of hydrogen and lithium atoms. The TDN2C method paves the way for the ab initio description of molecular spin transport and spintronics in the time domain.
Ab initio non-relativistic spin dynamics
NASA Astrophysics Data System (ADS)
Ding, Feizhi; Goings, Joshua J.; Frisch, Michael J.; Li, Xiaosong
2014-12-01
Many magnetic materials do not conform to the (anti-)ferromagnetic paradigm where all electronic spins are aligned to a global magnetization axis. Unfortunately, most electronic structure methods cannot describe such materials with noncollinear electron spin on account of formally requiring spin alignment. To overcome this limitation, it is necessary to generalize electronic structure methods and allow each electron spin to rotate freely. Here, we report the development of an ab initio time-dependent non-relativistic two-component spinor (TDN2C), which is a generalization of the time-dependent Hartree-Fock equations. Propagating the TDN2C equations in the time domain allows for the first-principles description of spin dynamics. A numerical tool based on the Hirshfeld partitioning scheme is developed to analyze the time-dependent spin magnetization. In this work, we also introduce the coupling between electron spin and a homogenous magnetic field into the TDN2C framework to simulate the response of the electronic spin degrees of freedom to an external magnetic field. This is illustrated for several model systems, including the spin-frustrated Li3 molecule. Exact agreement is found between numerical and analytic results for Larmor precession of hydrogen and lithium atoms. The TDN2C method paves the way for the ab initio description of molecular spin transport and spintronics in the time domain.
Dynamics of a Slender Spinning Membrane
NASA Astrophysics Data System (ADS)
Juang, Jer-Nan; Hung, Chung-Han; Wilkie, William K.
2013-12-01
A novel approach is introduced to conduct dynamic analysis of a spinning, high aspect ratio membrane. In this formulation, an inextensible, long, slender membrane is modeled using a discrete set of lumped masses. Lagranges equations are used to derive the highly coupled ordinary differential equations for in-plane, out-of-plane, and twisting motions for the spinning membrane. The generalized and uncoupled linear equations for small motion are used to compute the vibration mode frequencies which are compared to results from an uncoupled analysis of blade motion using rotor dynamics. Linearized behavior is shown to reduce to the linearized solutions for the spinning membrane blade developed by MacNeal. Numerical simulations along with 3-D animations are used to study the linear and nonlinear uncoupled dynamics of the spinning membrane.
NASA Astrophysics Data System (ADS)
Cheng, Lan; Gauss, Jürgen; Stanton, John F.
2013-08-01
A cost-effective treatment of scalar-relativistic effects on nuclear magnetic shieldings based on the spin-free exact-two-component theory in its one-electron variant (SFX2C-1e) is presented. The SFX2C-1e scheme gains its computational efficiency, in comparison to the four-component approach, from a focus on spin-free contributions and from the elimination of the small component. For the calculation of nuclear magnetic shieldings, the separation of spin-free and spin-dependent terms in the parent four-component theory is carried out here for the matrix representation of the Dirac equation in terms of a restricted-magnetically balanced gauge-including atomic orbital basis. The resulting spin-free four-component matrix elements required to calculate nuclear magnetic shieldings are then used to construct the corresponding SFX2C-1e Hamiltonian and its perturbed counterpart in the context of SFX2C-1e analytic derivative theory. To demonstrate the applicability of the approach, we report coupled-cluster calculations for prototypical problems such as the 17O shieldings of transition-metal oxo complexes (MO_4^{2-}, M = Cr, Mo, and W) and the 129Xe shieldings of xenon fluorides (XeF2, XeF4, and XeF6).
Aucar, I Agustín; Gomez, Sergio S; Giribet, Claudia G; Aucar, Gustavo A
2016-08-24
One of the most influential articles showing the best way to get the absolute values of NMR magnetic shieldings, σ (non-measurables) from both accurate measurements and theoretical calculations, was published a long time ago by Flygare. His model was shown to break down when heavy atoms are involved. This fact motivated the development of new theories of nuclear spin-rotation (SR) tensors, which consider electronic relativistic effects. One was published recently by some of us. In this article we take another step further and propose three different models that generalize Flygare's model. All of them are written using four-component relativistic expressions, though the two-component relativistic SO-S term also appears in one. The first clues for these developments were built from the relationship among σ and the SR tensors within the two-component relativistic LRESC model. Besides, we had to introduce a few other well defined assumptions: (i) relativistic corrections must be included in a way to best reproduce the relationship among the (e-e) term (called "paramagnetic" within the non-relativistic domain) of σ and its equivalent part of the SR tensor, (ii) as happens in Flygare's rule, the shielding of free atoms shall be included to improve accuracy. In the highest accurate model, a new term known as Spin-orbit due to spin, SO-S (in this mechanism the spin-Zeeman Hamiltonian replaces the orbital-Zeeman Hamiltonian), is included. We show the results of the application of those models to halogen containing linear molecules. PMID:27506822
Magnetic Suspension for Dynamic Spin Rig
NASA Technical Reports Server (NTRS)
Johnson, Dexter
1998-01-01
NASA Lewis Research Center's Dynamic Spin Rig, located in Building 5, Test Cell CW-18, is used to test turbomachinery blades and components by rotating them in a vacuum chamber. A team from Lewis' Machine Dynamics Branch successfully integrated a magnetic bearing and control system into the Dynamic Spin Rig. The magnetic bearing worked very well both to support and shake the shaft. It was demonstrated that the magnetic bearing can transmit more vibrational energy into the shaft and excite some blade modes to larger amplitudes than the existing electromagnetic shakers can.
Atomistic spin dynamics and surface magnons.
Etz, Corina; Bergqvist, Lars; Bergman, Anders; Taroni, Andrea; Eriksson, Olle
2015-06-24
Atomistic spin dynamics simulations have evolved to become a powerful and versatile tool for simulating dynamic properties of magnetic materials. It has a wide range of applications, for instance switching of magnetic states in bulk and nano-magnets, dynamics of topological magnets, such as skyrmions and vortices and domain wall motion. In this review, after a brief summary of the existing investigation tools for the study of magnons, we focus on calculations of spin-wave excitations in low-dimensional magnets and the effect of relativistic and temperature effects in such structures. In general, we find a good agreement between our results and the experimental values. For material specific studies, the atomistic spin dynamics is combined with electronic structure calculations within the density functional theory from which the required parameters are calculated, such as magnetic exchange interactions, magnetocrystalline anisotropy, and Dzyaloshinskii-Moriya vectors. PMID:26030259
Spinning compact binary dynamics and chameleon orbits
NASA Astrophysics Data System (ADS)
Gergely, László Árpád; Keresztes, Zoltán
2015-01-01
We analyze the conservative evolution of spinning compact binaries to second post-Newtonian (2PN) order accuracy, with leading-order spin-orbit, spin-spin and mass quadrupole-monopole contributions included. As a main result we derive a closed system of first-order differential equations in a compact form, for a set of dimensionless variables encompassing both orbital elements and spin angles. These evolutions are constrained by conservation laws holding at 2PN order. As required by the generic theory of constrained dynamical systems we perform a consistency check and prove that the constraints are preserved by the evolution. We apply the formalism to show the existence of chameleon orbits, whose local, orbital parameters evolve from elliptic (in the Newtonian sense) near pericenter, towards hyperbolic at large distances. This behavior is consistent with the picture that general relativity predicts stronger gravity at short distances than Newtonian theory does.
Fine-tuning the etch depth profile via dynamic shielding of ion beam
NASA Astrophysics Data System (ADS)
Wu, Lixiang; Qiu, Keqiang; Fu, Shaojun
2016-08-01
We introduce a method for finely adjusting the etch depth profile by dynamic shielding in the course of ion beam etching (IBE), which is crucial for the ultra-precision fabrication of large optics. We study the physical process of dynamic shielding and propose a parametric modeling method to quantitatively analyze the shielding effect on etch depths, or rather the shielding rate, where a piecewise Gaussian model is adopted to fit the shielding rate profile. Two experiments were conducted. The experimental result of parametric modeling of shielding rate profiles shows that the shielding rate profile is significantly influenced by the rotary angle of the leaf. The result of the experiment on fine-tuning the etch depth profile shows good agreement with the simulated result, which preliminarily verifies the feasibility of our method.
Dynamic magnetic shield for the CLAS12 central TOF detector photomultiplier tubes
2012-02-01
The Central Time-of-Flight detector for the Jefferson Laboratory 12-GeV upgrade is being designed with linear-focused photomultiplier tubes that require a robust magnetic shield against the CLAS12 main 5-T solenoid fringe fields of 100 mT (1 kG). Theoretical consideration of a ferromagnetic cylinder in an axial field has demonstrated that its shielding capability decreases with increasing length. This observation has been confirmed with finite element analysis using Poisson model software. Several shields composed of coaxial ferromagnetic cylinders have been studied. All difficulties caused by saturation effects were overcome with a novel dynamical shield, which utilizes a demagnetizing solenoid between the shielding cylinders. Basic dynamical shields for ordinary linear-focused 2-in. photomultiplier tubes were designed and tested both with models and experimental prototypes at different external field and demagnetizing current values. Our shield design reduces the 1 kG external axial field by a factor of 5000.
Kawasaki Dynamics on Bidimensional Spin Systems
NASA Astrophysics Data System (ADS)
Resende, Denilson C.; Cacüador, Felipe C.; Dantas, Sócrates O.
Under the influence of an external field many systems exhibit slow relaxations processes. In that sense, we study the Physics of this behavior/process in the early stages of its evolution on bidimensional Ising systems using Monte Carlo simulations at a broad range of temperature and spins up concentration. The Monte Carlo simulations were done up to second neighbors interactions shown a more stable dynamic regime than first neighbors interactions, when the systems energy is considered. The behavior of relative energy/spin and the relative perimeter (the line between spin up and spin down regions) are monitored against Monte Carlo steps. Also, our findings show that the stretching index (a2) exhibit values below the borderline (1) in a broad range of concentration below 50% and temperature from 0.5 ≤T ≤ 4.5 (in units of J/kB , where J is the ferromagnetic constant and kB is the Boltzmann constant).
The classical and quantum dynamics of molecular spins on graphene.
Cervetti, Christian; Rettori, Angelo; Pini, Maria Gloria; Cornia, Andrea; Repollés, Ana; Luis, Fernando; Dressel, Martin; Rauschenbach, Stephan; Kern, Klaus; Burghard, Marko; Bogani, Lapo
2016-02-01
Controlling the dynamics of spins on surfaces is pivotal to the design of spintronic and quantum computing devices. Proposed schemes involve the interaction of spins with graphene to enable surface-state spintronics and electrical spin manipulation. However, the influence of the graphene environment on the spin systems has yet to be unravelled. Here we explore the spin-graphene interaction by studying the classical and quantum dynamics of molecular magnets on graphene. Whereas the static spin response remains unaltered, the quantum spin dynamics and associated selection rules are profoundly modulated. The couplings to graphene phonons, to other spins, and to Dirac fermions are quantified using a newly developed model. Coupling to Dirac electrons introduces a dominant quantum relaxation channel that, by driving the spins over Villain's threshold, gives rise to fully coherent, resonant spin tunnelling. Our findings provide fundamental insight into the interaction between spins and graphene, establishing the basis for electrical spin manipulation in graphene nanodevices. PMID:26641019
The classical and quantum dynamics of molecular spins on graphene
NASA Astrophysics Data System (ADS)
Cervetti, Christian; Rettori, Angelo; Pini, Maria Gloria; Cornia, Andrea; Repollés, Ana; Luis, Fernando; Dressel, Martin; Rauschenbach, Stephan; Kern, Klaus; Burghard, Marko; Bogani, Lapo
2016-02-01
Controlling the dynamics of spins on surfaces is pivotal to the design of spintronic and quantum computing devices. Proposed schemes involve the interaction of spins with graphene to enable surface-state spintronics and electrical spin manipulation. However, the influence of the graphene environment on the spin systems has yet to be unravelled. Here we explore the spin-graphene interaction by studying the classical and quantum dynamics of molecular magnets on graphene. Whereas the static spin response remains unaltered, the quantum spin dynamics and associated selection rules are profoundly modulated. The couplings to graphene phonons, to other spins, and to Dirac fermions are quantified using a newly developed model. Coupling to Dirac electrons introduces a dominant quantum relaxation channel that, by driving the spins over Villain’s threshold, gives rise to fully coherent, resonant spin tunnelling. Our findings provide fundamental insight into the interaction between spins and graphene, establishing the basis for electrical spin manipulation in graphene nanodevices.
NASA Astrophysics Data System (ADS)
Soltner, Helmut; Pabst, Ulrich; Butzek, Michael; Ohl, Michael; Kozielewski, Tadeusz; Monkenbusch, Michael; Sokol, Don; Maltin, Larry; Lindgren, Eric; Koch, Stuart; Fugate, David
2011-07-01
A double-layer magnetically shielded room (MSR) has been designed and constructed for the neutron spin echo (NSE) spectrometer at the Spallation Neutron Source (SNS) in Oak Ridge, Tennessee. The primary objective of the MSR is to ensure an undisturbed operation of the spectrometer in terms of external magnetic fields from high-field magnets at neighboring beamlines and from other external devices. Because of the required mobility of the spectrometer along its beamline the MSR features a total length of about 17 m, which makes it the largest MSR worldwide. Several physics and engineering aspects addressed in the design phase and during the construction of this unique MSR are described in this article.
Unusual spin dynamics in topological insulators
Dóra, Balázs; Simon, Ferenc
2015-01-01
The dynamic spin susceptibility (DSS) has a ubiquitous Lorentzian form around the Zeeman energy in conventional materials with weak spin orbit coupling, whose spectral width characterizes the spin relaxation rate. We show that DSS has an unusual non-Lorentzian form in topological insulators, which are characterized by strong SOC, and the anisotropy of the DSS reveals the orientation of the underlying spin texture of topological states. At zero temperature, the high frequency part of DSS is universal and increases in certain directions as ωd−1 with d = 2 and 3 for surface states and Weyl semimetals, respectively, while for helical edge states, the interactions renormalize the exponent as d = 2K − 1 with K the Luttinger-liquid parameter. As a result, spin relaxation rate cannot be deduced from the DSS in contrast to the case of usual metals, which follows from the strongly entangled spin and charge degrees of freedom in these systems. PMID:26439629
Structurally Dynamic Spin Market Networks
NASA Astrophysics Data System (ADS)
Horváth, Denis; Kuscsik, Zoltán
The agent-based model of stock price dynamics on a directed evolving complex network is suggested and studied by direct simulation. The stationary regime is maintained as a result of the balance between the extremal dynamics, adaptivity of strategic variables and reconnection rules. The inherent structure of node agent "brain" is modeled by a recursive neural network with local and global inputs and feedback connections. For specific parametric combination the complex network displays small-world phenomenon combined with scale-free behavior. The identification of a local leader (network hub, agent whose strategies are frequently adapted by its neighbors) is carried out by repeated random walk process through network. The simulations show empirically relevant dynamics of price returns and volatility clustering. The additional emerging aspects of stylized market statistics are Zipfian distributions of fitness.
Topologically protected dynamics of spin textures
NASA Astrophysics Data System (ADS)
Tretiakov, O. A.; Abanov, Ar.
2015-06-01
We study current-induced dynamics of spin textures in thin magnetic nanowires. We derive effective equations of motion describing the dynamics of the domain-wall soft modes associated with topological defects. Because the magnetic domain walls are topological objects, these equations are universal and depend only on a few parameters. We obtain spin spiral domain-wall structure in ferromagnetic wires with Dzyaloshinskii-Moriya interaction and critical current dependence on this interaction. We also find the most efficient way to move the domain walls by resonant current pulses and propose a procedure to determine their dynamics by measuring the voltage induced by a moving domain wall. Based on translationally non-invariant nanowires, we show how to make prospective magnetic memory nanodevices much more energy efficient.
Dynamic Feedback in Ferromagnet-Spin Hall Metal Heterostructures.
Cheng, Ran; Zhu, Jian-Gang; Xiao, Di
2016-08-26
In ferromagnet-normal-metal heterostructures, spin pumping and spin-transfer torques are two reciprocal processes that occur concomitantly. Their interplay introduces a dynamic feedback effect interconnecting energy dissipation channels of both magnetization and current. By solving the spin diffusion process in the presence of the spin Hall effect in the normal metal, we show that the dynamic feedback gives rise to (i) a nonlinear magnetic damping that is crucial to sustain uniform steady-state oscillations of a spin Hall oscillator at large angles and (ii) a frequency-dependent spin Hall magnetoimpedance that reduces to the spin Hall magnetoresistance in the dc limit. PMID:27610880
Combined molecular dynamics-spin dynamics simulations of bcc iron
Perera, Meewanage Dilina N; Yin, Junqi; Landau, David P; Nicholson, Don M; Stocks, George Malcolm; Eisenbach, Markus; Brown, Greg
2014-01-01
Using a classical model that treats translational and spin degrees of freedom on an equal footing, we study phonon-magnon interactions in BCC iron with combined molecular and spin dynamics methods. The atomic interactions are modeled via an empirical many-body potential while spin dependent interactions are established through a Hamiltonian of the Heisenberg form with a distance dependent magnetic exchange interaction obtained from first principles electronic structure calculations. The temporal evolution of translational and spin degrees of freedom was determined by numerically solving the coupled equations of motion, using an algorithm based on the second order Suzuki-Trotter decomposition of the exponential operators. By calculating Fourier transforms of space- and time-displaced correlation functions, we demonstrate that the the presence of lattice vibrations leads to noticeable softening and damping of spin wave modes. As a result of the interplay between lattice and spin subsystems, we also observe additional longitudinal spin wave excitations, with frequencies which coincide with that of the longitudinal lattice vibrations.
Spin dynamics under local gauge fields in chiral spin-orbit coupling systems
NASA Astrophysics Data System (ADS)
Tan, S. G.; Jalil, M. B. A.; Fujita, T.; Liu, X. J.
2011-02-01
We present a theoretical description of local spin dynamics in magnetic systems with a chiral spin texture and finite spin-orbit coupling (SOC). Spin precession about the relativistic effective magnetic field in a SOC system gives rise to a non-Abelian SU(2) gauge field reminiscent of the Yang-Mills field. In addition, the adiabatic relaxation of electron spin along the local spin yields an U(1) ⊗ U(1) topological gauge (Berry) field. We derive the corresponding equation of motion i.e. modified Landau-Lifshitz-Gilbert (LLG) equation, for the local spin under the influence of these effects. Focusing on the SU(2) gauge, we obtain the spin torque magnitude, and the amplitude and frequency of spin oscillations in this system. Our theoretical estimates indicate significant spin torque and oscillations in systems with large spin-orbit coupling, which may be utilized in technological applications such as current-induced magnetization-switching and tunable microwave oscillators.
Spin glass dynamics at the mesoscale
NASA Astrophysics Data System (ADS)
Guchhait, Samaresh; Kenning, Gregory G.; Orbach, Raymond L.; Rodriguez, Gilberto F.
2015-01-01
The mesoscale allows a new probe of spin glass dynamics. Because the spin glass lower critical dimension dl>2 , the growth of the correlation length ξ (t ,T ) can change the nature of the spin glass state at a crossover time tco when ξ (tco,T )=ℓ , a minimum characteristic sample length (e.g., film thickness for thin films and crystallite size for bulk samples). For thin films, and times t
Nozirov, Farhod E-mail: farhod.nozirov@gmail.com; Stachów, Michał; Kupka, Teobald E-mail: farhod.nozirov@gmail.com
2014-04-14
A theoretical prediction of nuclear magnetic shieldings and indirect spin-spin coupling constants in 1,1-, cis- and trans-1,2-difluoroethylenes is reported. The results obtained using density functional theory (DFT) combined with large basis sets and gauge-independent atomic orbital calculations were critically compared with experiment and conventional, higher level correlated electronic structure methods. Accurate structural, vibrational, and NMR parameters of difluoroethylenes were obtained using several density functionals combined with dedicated basis sets. B3LYP/6-311++G(3df,2pd) optimized structures of difluoroethylenes closely reproduced experimental geometries and earlier reported benchmark coupled cluster results, while BLYP/6-311++G(3df,2pd) produced accurate harmonic vibrational frequencies. The most accurate vibrations were obtained using B3LYP/6-311++G(3df,2pd) with correction for anharmonicity. Becke half and half (BHandH) density functional predicted more accurate {sup 19}F isotropic shieldings and van Voorhis and Scuseria's τ-dependent gradient-corrected correlation functional yielded better carbon shieldings than B3LYP. A surprisingly good performance of Hartree-Fock (HF) method in predicting nuclear shieldings in these molecules was observed. Inclusion of zero-point vibrational correction markedly improved agreement with experiment for nuclear shieldings calculated by HF, MP2, CCSD, and CCSD(T) methods but worsened the DFT results. The threefold improvement in accuracy when predicting {sup 2}J(FF) in 1,1-difluoroethylene for BHandH density functional compared to B3LYP was observed (the deviations from experiment were −46 vs. −115 Hz)
Lindblad dynamics of a quantum spherical spin
NASA Astrophysics Data System (ADS)
Wald, Sascha; Henkel, Malte
2016-03-01
The coherent quantum dynamics of a single bosonic spin variable, subject to a constraint derived from the quantum spherical model of a ferromagnet, and coupled to an external heat bath, is studied through the Lindblad equation for the reduced density matrix. Closed systems of equations of motion for several quantum observables are derived and solved exactly. The relationship to the single-mode Dicke model from quantum optics is discussed. The analysis of the interplay of the quantum fluctuation and the dissipation and their influence on the relaxation of the time-dependent magnetisation leads to the distinction of qualitatively different regimes of weak and strong quantum couplings. Considering the model’s behaviour in an external field as a simple mean-field approximation of the dynamics of a quantum spherical ferromagnet, the magnetic phase diagram appears to be re-entrant and presents a quantum analogue of well-established classical examples of fluctuation-induced order.
NMR shielding and spin-rotation constants of 175LuX (X = 19F, 35Cl, 79Br, 127I) molecules
NASA Astrophysics Data System (ADS)
Demissie, Taye B.
2015-12-01
This presentation demonstrates the relativistic effects on the spin-rotation constants, absolute nuclear magnetic resonance (NMR) shielding constants and shielding spans of 175LuX (X = 19F, 35Cl, 79Br, 127I) molecules. The results are obtained from calculations performed using density functional theory (non-relativistic and four-component relativistic) and coupled-cluster calculations. The spin-rotation constants are compared with available experimental values. In most of the molecules studied, relativistic effects make an order of magnitude difference on the NMR absolute shielding constants.
Dynamic Open-Rotor Composite Shield Impact Test Report
NASA Technical Reports Server (NTRS)
Seng, Silvia; Frankenberger, Charles; Ruggeri, Charles R.; Revilock, Duane M.; Pereira, J. Michael; Carney, Kelly S.; Emmerling, William C.
2015-01-01
The Federal Aviation Administration (FAA) is working with the European Aviation Safety Agency to determine the certification base for proposed new engines that would not have a containment structure on large commercial aircraft. Equivalent safety to the current fleet is desired by the regulators, which means that loss of a single fan blade will not cause hazard to the aircraft. NASA Glenn and Naval Air Warfare Center (NAWC) China Lake collaborated with the FAA Aircraft Catastrophic Failure Prevention Program to design and test a shield that would protect the aircraft passengers and critical systems from a released blade that could impact the fuselage. This report documents the live-fire test from a full-scale rig at NAWC China Lake. NASA provided manpower and photogrammetry expertise to document the impact and damage to the shields. The test was successful: the blade was stopped from penetrating the shield, which validates the design analysis method and the parameters used in the analysis. Additional work is required to implement the shielding into the aircraft.
Nonequilibrium dynamics and spin segregation in trapped gases
NASA Astrophysics Data System (ADS)
Koller, Andrew P.; Mundinger, Joshua; Wall, Michael L.; Rey, Ana Maria
2015-05-01
We consider harmonically trapped spin-1/2 gases quenched far from equilibrium by a Ramsey pulse. A magnetic field gradient is applied to the trapped gas, resulting in different trapping potentials for the two spin species. We model the dynamics using an effective spin model Hamiltonian with long range interactions, and use the spin model to understand the results of several experiments on spin diffusion and spin segregation in trapped gases. Supported by JILA-NSF-PFC-1125844, NSF-PIF- 1211914, ARO, AFOSR, AFOSR-MURI, and NDSEG.
Dynamic Stabilization of a Quantum Many-Body Spin System
NASA Astrophysics Data System (ADS)
Hoang, T. M.; Gerving, C. S.; Land, B. J.; Anquez, M.; Hamley, C. D.; Chapman, M. S.
2013-08-01
We demonstrate dynamic stabilization of a strongly interacting quantum spin system realized in a spin-1 atomic Bose-Einstein condensate. The spinor Bose-Einstein condensate is initialized to an unstable fixed point of the spin-nematic phase space, where subsequent free evolution gives rise to squeezing and quantum spin mixing. To stabilize the system, periodic microwave pulses are applied that rotate the spin-nematic many-body fluctuations and limit their growth. The stability diagram for the range of pulse periods and phase shifts that stabilize the dynamics is measured and compares well with a stability analysis.
Dynamic stabilization of a quantum many-body spin system.
Hoang, T M; Gerving, C S; Land, B J; Anquez, M; Hamley, C D; Chapman, M S
2013-08-30
We demonstrate dynamic stabilization of a strongly interacting quantum spin system realized in a spin-1 atomic Bose-Einstein condensate. The spinor Bose-Einstein condensate is initialized to an unstable fixed point of the spin-nematic phase space, where subsequent free evolution gives rise to squeezing and quantum spin mixing. To stabilize the system, periodic microwave pulses are applied that rotate the spin-nematic many-body fluctuations and limit their growth. The stability diagram for the range of pulse periods and phase shifts that stabilize the dynamics is measured and compares well with a stability analysis. PMID:24033006
Nonequilibrium Spin Dynamics: from Protons in Water to a Gauge Theory of Spin-Orbit Coupling
NASA Astrophysics Data System (ADS)
Tokatly, I. V.; Sherman, E. Ya.
Nonequilibrium dynamics of spin degrees of freedom in condensed matter, ranging from classical liquids to solids and ultracold atomic gases, is one of the focus topics in physics. Here we present a gauge theory of spin dynamics in spinorbit coupled gases for a "pure" gauge realization of the spin-orbit coupling field. This approach allows one to describe the spin dynamics in fermionic systems in terms of exact general response functions and to map it on the density dynamics in a dual system without spin-orbit coupling. We apply this approach to electrons in disordered two-dimensional structures and to cold atomic gases of interacting fermions with synthetic spin-orbit coupling at very low temperatures.
Photoexcited carrier spin dynamics in CH3NH
NASA Astrophysics Data System (ADS)
Odenthal, Patrick; Gundlach, Nathan; Talmadge, William; Wang, Ruizhi; Zhang, Chuang; Sun, Dali; Vardeny, Zeev Valy; Li, Yan (Sarah)
Metal halide perovskites have shown great promise for the field of spintronics due to their large tunable spin-orbit coupling, spin dependent optical selection rules and predicted electrically tunable Rashba band. The spin sensitive optical transitions allow optical spin orientation of carriers using circularly polarized light, and detection of the spin polarization via optical Faraday rotation measurement. We study carrier spin dynamics on solution-processed polycrystalline CH3NH3PbI3 films using time-resolved Faraday rotation (TRFR). TRFR reveals unexpected long spin lifetimes exceeding 1ns at 4K. This is significant given that Pb and I exhibit large spin-orbit coupling, which usually lead to fast spin relaxation. Research supported by the NSF-MRSEC (DMR 1121252) at the University of Utah.
Spin-orbit effects on the (119)Sn magnetic-shielding tensor in solids: a ZORA/DFT investigation.
Alkan, Fahri; Holmes, Sean T; Iuliucci, Robbie J; Mueller, Karl T; Dybowski, Cecil
2016-07-28
Periodic-boundary and cluster calculations of the magnetic-shielding tensors of (119)Sn sites in various co-ordination and stereochemical environments are reported. The results indicate a significant difference between the predicted NMR chemical shifts for tin(ii) sites that exhibit stereochemically-active lone pairs and tin(iv) sites that do not have stereochemically-active lone pairs. The predicted magnetic shieldings determined either with the cluster model treated with the ZORA/Scalar Hamiltonian or with the GIPAW formalism are dependent on the oxidation state and the co-ordination geometry of the tin atom. The inclusion of relativistic effects at the spin-orbit level removes systematic differences in computed magnetic-shielding parameters between tin sites of differing stereochemistries, and brings computed NMR shielding parameters into significant agreement with experimentally-determined chemical-shift principal values. Slight improvement in agreement with experiment is noted in calculations using hybrid exchange-correlation functionals. PMID:27354312
The classical and quantum dynamics of molecular spins on graphene
Cervetti, Christian; Rettori, Angelo; Pini, Maria Gloria; Cornia, Andrea; Repollés, Ana; Luis, Fernando; Dressel, Martin; Rauschenbach, Stephan; Kern, Klaus; Burghard, Marko; Bogani, Lapo
2015-01-01
Controlling the dynamics of spins on surfaces is pivotal to the design of spintronic1 and quantum computing2 devices. Proposed schemes involve the interaction of spins with graphene to enable surface-state spintronics3,4, and electrical spin-manipulation4-11. However, the influence of the graphene environment on the spin systems has yet to be unraveled12. Here we explore the spin-graphene interaction by studying the classical and quantum dynamics of molecular magnets13 on graphene. While the static spin response remains unaltered, the quantum spin dynamics and associated selection rules are profoundly modulated. The couplings to graphene phonons, to other spins, and to Dirac fermions are quantified using a newly-developed model. Coupling to Dirac electrons introduces a dominant quantum-relaxation channel that, by driving the spins over Villain’s threshold, gives rise to fully-coherent, resonant spin tunneling. Our findings provide fundamental insight into the interaction between spins and graphene, establishing the basis for electrical spin-manipulation in graphene nanodevices. PMID:26641019
SD-CAS: Spin Dynamics by Computer Algebra System.
Filip, Xenia; Filip, Claudiu
2010-11-01
A computer algebra tool for describing the Liouville-space quantum evolution of nuclear 1/2-spins is introduced and implemented within a computational framework named Spin Dynamics by Computer Algebra System (SD-CAS). A distinctive feature compared with numerical and previous computer algebra approaches to solving spin dynamics problems results from the fact that no matrix representation for spin operators is used in SD-CAS, which determines a full symbolic character to the performed computations. Spin correlations are stored in SD-CAS as four-entry nested lists of which size increases linearly with the number of spins into the system and are easily mapped into analytical expressions in terms of spin operator products. For the so defined SD-CAS spin correlations a set of specialized functions and procedures is introduced that are essential for implementing basic spin algebra operations, such as the spin operator products, commutators, and scalar products. They provide results in an abstract algebraic form: specific procedures to quantitatively evaluate such symbolic expressions with respect to the involved spin interaction parameters and experimental conditions are also discussed. Although the main focus in the present work is on laying the foundation for spin dynamics symbolic computation in NMR based on a non-matrix formalism, practical aspects are also considered throughout the theoretical development process. In particular, specific SD-CAS routines have been implemented using the YACAS computer algebra package (http://yacas.sourceforge.net), and their functionality was demonstrated on a few illustrative examples. PMID:20843716
Gryff-Keller, Adam; Kraska-Dziadecka, Anna; Molchanov, Sergey; Wodyński, Artur
2012-11-01
Magnetic shielding and indirect spin-spin coupling phenomena are tensorial properties and both their isotropic and anisotropic parts do affect NMR spectra. The involved interaction tensors, σ and J, can nowadays be theoretically calculated, although the reliability of such methods in the case of anisotropic parameters, Δσ and ΔJ, in systems involving heavy nuclei, yet demands testing. In this communication the results of the experimental and theoretical investigations of bis(phenylethynyl)mercury (I) labeled with (13)C isotope at positions neighboring Hg are reported. The theoretical calculations of molecular geometry and values of NMR parameters for I have been performed by the ZORA/DFT method, including the relativistic scalar and spin-orbit coupling contributions, using the PBE0 functional and TZP (or jcpl) basis set. These values have been confronted with the experimentally measured ones. The isotropic parameters have been measured by the standard (13)C and (199)Hg NMR spectra. The shielding anisotropies for the atoms in the central part of molecule I have been determined in a liquid sample using magnetic relaxation measurements. The relaxation data have been interpreted within the rotational diffusion theory, assuming the symmetrical top reorientation model. The anisotropies of one-bond (13)C-(199)Hg and two-bond (13)C-Hg-(13)C spin-spin couplings have been determined exploiting the temperature-dependent (13)C NMR spectra of I in the ZLI1167 liquid-crystal phase. We have found that our theoretical calculations reproduce experimental values of both isotropic and anisotropic NMR parameters very well. PMID:23050748
Dynamical analysis of a spinning solar sail
NASA Astrophysics Data System (ADS)
Gong, Shengping; Li, Junfeng; Zhu, Kaijian
2011-12-01
This paper discusses the orbit and attitude dynamics of a solar sail, and gives the sufficient conditions of a stable orbit and attitude coupled system. The stability of the coupled system is determined by the orbit stability and attitude stability. Based on the sufficient conditions, a spin-stabilized solar sail of cone configuration is proposed to evolve in the heliocentric displaced orbit. For this kind of configuration, the attitude is always stable by spinning itself. The orbit stability depends on the orbit parameters of the heliocentric displaced orbit, the ratio of the orbit radius to displaced distance and orbit angular velocity. If the center of mass and center of pressure overlap, it can be proved that the coupled system is stable when the orbit parameters are chosen in the stable region. When the center of mass and center of pressure offset exists, the stability of the coupled system can not be judged. A numerical example is given and the result shows that both the orbit and attitude are stable for the case.
Low-Energy Spin Dynamics of the Honeycomb Spin Liquid Beyond the Kitaev Limit
NASA Astrophysics Data System (ADS)
Song, Xue-Yang; You, Yi-Zhuang; Balents, Leon
2016-07-01
We investigate the generic features of the low energy dynamical spin structure factor of the Kitaev honeycomb quantum spin liquid perturbed away from its exact soluble limit by generic symmetry-allowed exchange couplings. We find that the spin gap persists in the Kitaev-Heisenberg model, but generally vanishes provided more generic symmetry-allowed interactions exist. We formulate the generic expansion of the spin operator in terms of fractionalized Majorana fermion operators according to the symmetry enriched topological order of the Kitaev spin liquid, described by its projective symmetry group. The dynamical spin structure factor displays power-law scaling bounded by Dirac cones in the vicinity of the Γ , K , and K' points of the Brillouin zone, rather than the spin gap found for the exactly soluble point.
Influences of Initial States on Entanglement Dynamics of Two Central Spins in a Spin Environment
NASA Astrophysics Data System (ADS)
Yu, Wen-Jian; Xu, Bao-Ming; Li, Lin; Zou, Jian; Li, Hai; Shao, Bin
2016-03-01
We investigate the entanglement dynamics of two electronic spins coupled to a bath of nuclear spins for two special cases, one is that two central spins both interact with a common bath, and the other is that one of two spins interacts with a bath. We consider three types of initial states with different correlations between the system and the bath, i.e., quantum correlation, classical correlation, and no-correlation. We show that the initial correlations (no matter quantum correlations or classical correlations) can effectively avoid the occurrence of entanglement sudden death. Irrespective of whether both two spins or only one of the two spins interacts with the bath, the system can gain more entanglement in the process of the time evolution for initial quantum correlations. In addition, we find that the effects of the distribution of coupling constants on entanglement dynamics crucially depend on the initial state of the spin bath.
Control of electron spin decoherence caused by electron nuclear spin dynamics in a quantum dot
NASA Astrophysics Data System (ADS)
Liu, Ren-Bao; Yao, Wang; Sham, L. J.
2007-07-01
Control of electron spin decoherence in contact with a mesoscopic bath of many interacting nuclear spins in an InAs quantum dot is studied by solving the coupled quantum dynamics. The nuclear spin bath, because of its bifurcated evolution predicated on the electron spin up or down state, measures the which-state information of the electron spin and hence diminishes its coherence. The many-body dynamics of the nuclear spin bath is solved with a pair-correlation approximation. In the relevant timescale, nuclear pair-wise flip flops, as elementary excitations in the mesoscopic bath, can be mapped into the precession of non-interacting pseudo-spins. Such mapping provides a geometrical picture for understanding the decoherence and for devising control schemes. A close examination of nuclear bath dynamics reveals a wealth of phenomena and new possibilities of controlling the electron spin decoherence. For example, when the electron spin is flipped by a π-pulse at τ, its coherence will partially recover at \\sqrt{2}\\tau as a consequence of quantum disentanglement from the mesoscopic bath. In contrast to the re-focusing of inhomogeneously broadened phases by conventional spin-echoes, the disentanglement is realized through shepherding quantum evolution of the bath state via control of the quantum object. A concatenated construction of pulse sequences can eliminate the decoherence with arbitrary accuracy, with the nuclear nuclear spin interaction strength acting as the controlling small parameter.
Dynamical Decoupling with pulse errors for ensembles of interacting spins
NASA Astrophysics Data System (ADS)
Petersen, E. S.; Tyryshkin, A. M.; Lyon, S. A.
Dynamical decoupling (DD) is a well-known approach for decoupling quantum (spin) systems from their environments. Theoretically, the performance of DD pulse sequences is often analyzed using a single spin approximation in which environmental noise is included through single spin operators. This approach has successfully analyzed the effectiveness of many popular DD pulse sequences (like CPMG and XY4) to cancel environmental noise even in the presence of unavoidable pulse errors. However, this methodology does not describe the effect of DD on the spin-spin interactions present in experiments involving large numbers of spins. Here, we go beyond the usual single-spin model, extending the analysis of DD sequences to include such spin-spin interactions. We find that when using certain popular DD sequences (like CPMG), coherence times of ensembles with dipolar interactions between spins can be drastically influenced by pulse errors. While sequences with ideal pulses do not decouple the spin-spin interactions, the presence of even small pulse errors can partially (or even greatly) decouple the spin-spin interactions thus leading to longer coherence times. Furthermore, the extent that these interactions are decoupled is highly dependent on the type of DD sequence used, and not necessarily the number of pulses involved. These calculations explain results of past experiments (Tyryshkin et al., arxiv: 1011.1903).
Electron-spin dynamics in elliptically polarized light waves
NASA Astrophysics Data System (ADS)
Bauke, Heiko; Ahrens, Sven; Grobe, Rainer
2014-11-01
We investigate the coupling of the spin angular momentum of light beams with elliptical polarization to the spin degree of freedom of free electrons. It is shown that this coupling, which is of similar origin as the well-known spin-orbit coupling, can lead to spin precession. The spin-precession frequency is proportional to the product of the laser field's intensity and its spin density. The electron-spin dynamics is analyzed by employing exact numerical methods as well as time-dependent perturbation theory based on the fully relativistic Dirac equation and on the nonrelativistic Pauli equation that is amended by a relativistic correction that accounts for the light's spin density.
Quantum dynamics of interacting spins mediated by phonons and photons
NASA Astrophysics Data System (ADS)
Senko, Crystal
2015-03-01
Techniques that enable robust, controllable interactions among quantum particles are now being actively explored. They constitute a key ingredient for quantum information processing and quantum simulations. We describe two atom-based platforms to experimentally realize and study quantum dynamics with controllable, long-range spin-spin interactions. Using trapped atomic ions, we implemented tunable spin-spin interactions mediated by optical dipole forces, which represent a new approach to study quantum magnetism. This platform has enabled sophisticated manipulations of more than 10 spins, and realization of quantum simulations of integer-spin chains. In a separate set of experiments we realized a hybrid system in which single photons, confined to sub-wavelength dimensions with a photonic crystal cavity, are coupled to single trapped neutral atoms. Extending this architecture to multiple atoms enables photon-induced quantum gates, and tunable spin-spin interactions, between distant atoms.
NASA Astrophysics Data System (ADS)
Zevenhoven, Koos C. J.; Dong, Hui; Ilmoniemi, Risto J.; Clarke, John
2015-01-01
Pulse-induced transients such as eddy currents can cause problems in measurement techniques where a signal is acquired after an applied preparatory pulse. In ultra-low-field magnetic resonance imaging, performed in magnetic fields typically of the order of 100 μT, the signal-to-noise ratio is enhanced in part by prepolarizing the proton spins with a pulse of much larger magnetic field and in part by detecting the signal with a Superconducting QUantum Interference Device (SQUID). The pulse turn-off, however, can induce large eddy currents in the shielded room, producing an inhomogeneous magnetic-field transient that both seriously distorts the spin dynamics and exceeds the range of the SQUID readout. It is essential to reduce this transient substantially before image acquisition. We introduce dynamical cancellation (DynaCan), a technique in which a precisely designed current waveform is applied to a separate coil during the later part and turn off of the polarizing pulse. This waveform, which bears no resemblance to the polarizing pulse, is designed to drive the eddy currents to zero at the precise moment that the polarizing field becomes zero. We present the theory used to optimize the waveform using a detailed computational model with corrections from measured magnetic-field transients. SQUID-based measurements with DynaCan demonstrate a cancellation of 99%. Dynamical cancellation has the great advantage that, for a given system, the cancellation accuracy can be optimized in software. This technique can be applied to both metal and high-permeability alloy shielded rooms, and even to transients other than eddy currents.
Zevenhoven, Koos C. J. Ilmoniemi, Risto J.; Dong, Hui; Clarke, John
2015-01-19
Pulse-induced transients such as eddy currents can cause problems in measurement techniques where a signal is acquired after an applied preparatory pulse. In ultra-low-field magnetic resonance imaging, performed in magnetic fields typically of the order of 100 μT, the signal-to-noise ratio is enhanced in part by prepolarizing the proton spins with a pulse of much larger magnetic field and in part by detecting the signal with a Superconducting QUantum Interference Device (SQUID). The pulse turn-off, however, can induce large eddy currents in the shielded room, producing an inhomogeneous magnetic-field transient that both seriously distorts the spin dynamics and exceeds the range of the SQUID readout. It is essential to reduce this transient substantially before image acquisition. We introduce dynamical cancellation (DynaCan), a technique in which a precisely designed current waveform is applied to a separate coil during the later part and turn off of the polarizing pulse. This waveform, which bears no resemblance to the polarizing pulse, is designed to drive the eddy currents to zero at the precise moment that the polarizing field becomes zero. We present the theory used to optimize the waveform using a detailed computational model with corrections from measured magnetic-field transients. SQUID-based measurements with DynaCan demonstrate a cancellation of 99%. Dynamical cancellation has the great advantage that, for a given system, the cancellation accuracy can be optimized in software. This technique can be applied to both metal and high-permeability alloy shielded rooms, and even to transients other than eddy currents.
Magnetization dynamics in exchange coupled antiferromagnet spin superfluids
NASA Astrophysics Data System (ADS)
Liu, Yizhou; Barlas, Yafis; Yin, Gen; Zang, Jiadong; Lake, Roger
Antiferromagnets (AFMs) are commonly used as the exchange bias layer in magnetic recording and spintronic devices. Recently, several studies on the spin transfer torque and spin pumping in AFMs reveal much more interesting physics in AFMs. Properties of AFMs such as the ultrafast switching within picoseconds and spin superfluidity demonstrate the potential to build AFM based spintronic devices. Here, we study the magnetization dynamics in an exchange coupled AFM systems. Beginning from the Landau-Lifshitz-Gilbert equation, we derive a Josephson-like equation for the exchange coupled system. We investigate the detailed magnetization dynamics by employing spin injection and spin pumping theory. We also propose a geometry that could be used to measure this magnetization dynamics. This work was supported as part of the Spins and Heat in Nanoscale Electronic Systems (SHINES) an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award #SC0012670.
Electron Spin Dynamics in Semiconductor Quantum Dots
Marie, X.; Belhadj, T.; Urbaszek, B.; Amand, T.; Krebs, O.; Lemaitre, A.; Voisin, P.
2011-07-15
An electron spin confined to a semiconductor quantum dot is not subject to the classical spin relaxation mechanisms known for free carriers but it strongly interacts with the nuclear spin system via the hyperfine interaction. We show in time resolved photoluminescence spectroscopy experiments on ensembles of self assembled InAs quantum dots in GaAs that this interaction leads to strong electron spin dephasing.
Static and dynamic elastic properties of rocks from the Canadian Shield
King, M.S.
1983-01-01
As part of a number of research studies in the Canadian Shield associated with the stability of underground mine openings, seismic reflection surveys, and the proposed use of a tunnel-boring machine (TBM) for developing mine headings, a long-term laboratory rock mechanics program has been conducted to determine the static and dynamic elastic properties of samples of igneous and metamorphic rocks from the Canadian Shield. This paper reports the results of 174 measurements of static elastic modulus and 152 measurements of uniaxial compressive strength for these rocks as a function of dynamic elastic modulus. 20 references, 5 figures.
Spin dynamics under local gauge fields in chiral spin-orbit coupling systems
Tan, S.G.; Jalil, M.B.A.; Fujita, T.; Liu, X.J.
2011-02-15
Research Highlights: > We derive a modified LLG equation in magnetic systems with spin-orbit coupling (SOC). > Our results are applied to magnetic multilayers, and DMS and magnetic Rashba systems. > SOC mediated magnetization switching is predicted in rare earth metals (large SOC). > The magnetization trajectory and frequency can be modulated by applied voltage. > This facilitates potential application as tunable microwave oscillators. - Abstract: We present a theoretical description of local spin dynamics in magnetic systems with a chiral spin texture and finite spin-orbit coupling (SOC). Spin precession about the relativistic effective magnetic field in a SOC system gives rise to a non-Abelian SU(2) gauge field reminiscent of the Yang-Mills field. In addition, the adiabatic relaxation of electron spin along the local spin yields an U(1) x U(1) topological gauge (Berry) field. We derive the corresponding equation of motion i.e. modified Landau-Lifshitz-Gilbert (LLG) equation, for the local spin under the influence of these effects. Focusing on the SU(2) gauge, we obtain the spin torque magnitude, and the amplitude and frequency of spin oscillations in this system. Our theoretical estimates indicate significant spin torque and oscillations in systems with large spin-orbit coupling, which may be utilized in technological applications such as current-induced magnetization-switching and tunable microwave oscillators.
Nonlinear dynamics of spin and charge in spin-Calogero model
Kulkarni, Manas; Franchini, Fabio; Abanov, Alexander G.
2009-10-15
The fully nonlinear dynamics of spin and charge in spin-Calogero model is studied. The latter is an integrable one-dimensional model of quantum spin-1/2 particles interacting through inverse-square interaction and exchange. Classical hydrodynamic equations of motion are written for this model in the regime where gradient corrections to the exact hydrodynamic formulation of the theory may be neglected. In this approximation variables separate in terms of dressed Fermi momenta of the model. Hydrodynamic equations reduce to a set of decoupled Riemann-Hopf (or inviscid Burgers') equations for the dressed Fermi momenta. We study the dynamics of some nonequilibrium spin-charge configurations for times smaller than the time scale of the gradient catastrophe. We find an interesting interplay between spin and charge degrees of freedom. In the limit of large coupling constant the hydrodynamics reduces to the spin hydrodynamics of the Haldane-Shastry model.
Electrical control of single spin dynamics
NASA Astrophysics Data System (ADS)
Petta, Jason
2012-02-01
Over ten years ago, Daniel Loss and David DiVincenzo proposed using the spin of a single electron as a quantum bit. At the time of the proposal, it was not possible to trap a single electron in a device and measure its spin, let alone demonstrate control of quantum coherence. In this talk I will describe recent progress in the field, focusing on two new methods for single spin control that have been developed by my group at Princeton. The first method is based on quantum interference and implements spin-interferometry on a chip. The second method utilizes the strong spin-orbit coupling of InAs. By shifting the orbital position of the electronic wavefunction at gigahertz frequencies, we can control the orientation of a single electron spin and measure the full g-tensor, which exhibits a large anisotropy due to spin-orbit interactions. Both methods for single spin control are orders of magnitude faster than conventional electron spin resonance and allow investigations of single spin coherence in the presence of fluctuating nuclear and spin-orbit fields. I will also describe recent efforts to transfer these methods to silicon quantum dots, where the effects of fluctuating nuclear fields are much smaller.
Dynamical aspects of spin chains at infinite temperature for different spin quantum numbers
NASA Astrophysics Data System (ADS)
Böhm, Markus; Leschke, Hajo
1993-10-01
For infinite temperature we exactly calculate the coefficients of the short-time expansion of the spin-pair correlations in one-dimensional spin models. For spin quantum numbers s = 1 we present the coefficients up to order t18 and t22, for classical spins up to order t16 and t18 for the isotropic Heisenberg chain and the isotropic XY-chain, respectively. These coefficients are used together with recently determined ones for s = {1}/{2} to compute bounds on the autocorrelation functions, to approximate the associated spectral densities and to bound the spatial variances of pair correlations. The results are compared with those obtained from simulation data of Gerling and Landau (Phys. Rev. B 42 (1990) 8214) for classical spin chains. Over the available time region, we find a rather smooth dependence of the dynamics on the spin quantum number and see some evidence for spin diffusion.
Semiclassical spin-spin dynamics and feedback control in transport through a quantum dot
NASA Astrophysics Data System (ADS)
Mosshammer, Klemens; Brandes, Tobias
2014-10-01
We present a theory of magnetotransport through an electronic orbital, where the electron spin interacts with a (sufficiently) large external spin via an exchange interaction. Using a semiclassical approximation, we derive a set of equations of motions for the electron density matrix and the mean value of the external spin that turns out to be highly nonlinear. The dissipation via the electronic leads is implemented in terms of a quantum master equation that is combined with the nonlinear terms of the spin-spin interaction. With an anisotropic exchange coupling a variety of dynamics is generated, such as self-sustained oscillations with parametric resonances or even chaotic behavior. Within our theory we can integrate a Maxwell-demon-like closed-loop feedback scheme that is capable of transporting particles against an applied bias voltage and that can be used to implement a spin filter to generate spin-dependent oscillating currents of opposite directions.
The Magnetic and Shielding Effects of Ring Current on Radiation Belt Dynamics
NASA Technical Reports Server (NTRS)
Fok, Mei-Ching
2012-01-01
The ring current plays many key roles in controlling magnetospheric dynamics. A well-known example is the magnetic depression produced by the ring current, which alters the drift paths of radiation belt electrons and may cause significant electron flux dropout. Little attention is paid to the ring current shielding effect on radiation belt dynamics. A recent simulation study that combines the Comprehensive Ring Current Model (CRCM) with the Radiation Belt Environment (RBE) model has revealed that the ring current-associated shielding field directly and/or indirectly weakens the relativistic electron flux increase during magnetic storms. In this talk, we will discuss how ring current magnetic field and electric shielding moderate the radiation belt enhancement.
Dynamics of Spin-(1)/(2) Quantum Plasmas
NASA Astrophysics Data System (ADS)
Marklund, Mattias; Brodin, Gert
2007-01-01
The fully nonlinear governing equations for spin-(1)/(2) quantum plasmas are presented. Starting from the Pauli equation, the relevant plasma equations are derived, and it is shown that nontrivial quantum spin couplings arise, enabling studies of the combined collective and spin dynamics. The linear response of the quantum plasma in an electron-ion system is obtained and analyzed. Applications of the theory to solid state and astrophysical systems as well as dusty plasmas are pointed out.
Dynamics of spin-1/2 quantum plasmas.
Marklund, Mattias; Brodin, Gert
2007-01-12
The fully nonlinear governing equations for spin-1/2 quantum plasmas are presented. Starting from the Pauli equation, the relevant plasma equations are derived, and it is shown that nontrivial quantum spin couplings arise, enabling studies of the combined collective and spin dynamics. The linear response of the quantum plasma in an electron-ion system is obtained and analyzed. Applications of the theory to solid state and astrophysical systems as well as dusty plasmas are pointed out. PMID:17358613
Dynamics of test bodies with spin in de Sitter spacetime
Obukhov, Yuri N.; Puetzfeld, Dirk
2011-02-15
We study the motion of spinning test bodies in the de Sitter spacetime of constant positive curvature. With the help of the 10 Killing vectors, we derive the 4-momentum and the tensor of spin explicitly in terms of the spacetime coordinates. However, in order to find the actual trajectories, one needs to impose the so-called supplementary condition. We discuss the dynamics of spinning test bodies for the cases of the Frenkel and Tulczyjew conditions.
NASA Astrophysics Data System (ADS)
Lazzeretti, P.; Malagoli, M.; Turci, L.; Zanasi, R.
1993-10-01
Theoretical methods based on the random-phase approximation have been applied to evaluate near Hartree-Fock dynamic electric polarizability and shielding tensors of carbon and hydrogen nuclei in the benzene molecule. Cauchy moments of the various properties have been determined. The results obtained in different gauges (dipole length, velocity, and acceleration) are reported.
Toward Ultrafast Spin Dynamics in Low Dimensional Semiconductors
NASA Astrophysics Data System (ADS)
Chiu, Yi-Hsin
Since the discovery of long spin relaxation times of itinerant electrons up to 100 nanoseconds and spin diffusion lengths over 100 mum in GaAs, extraordinary advances in semiconductor spintronics have been made in the past one and half decades. Incorporating spins in semiconductors requires the following essential capabilities: (i) injection of spins into semiconductors, (ii) manipulation of spins, and (iii) sensitive detection of spin coherence. The solutions to these challenges lie in a deeper understanding of spin interactions and spin relaxation in semiconductors as well as appropriate tools to probe spin dynamics. In particular, recent experiments have suggested the important role of dimensionality in spin dynamics. For example, spin-orbit interaction, the dominant source of spin relaxation in most II-VI and III-V semiconductors, has been shown to be significantly suppressed in reduced dimensions. Low-dimensional semiconductors are therefore appealing candidates for exploring spin physics and device applications. This dissertation aims at exploring spin dynamics in low dimensional semiconductor systems using time-resolved optical techniques. The time resolution allows for a direct measurement of the equilibrium and non-equilibrium carrier spins and various spin interactions in the time domain. Optical approaches are also a natural fit for probing optically active nanostructures where electric approaches can often encounter challenges. For instance, fabricating electric contacts with nanostructures is a proven challenge because of their reduced size and modified electronic structure. This dissertation is divided into three sections targeting an ultimate goal of employing optical methods to explore spin dynamics in low dimensional semiconductors. First, the time-resolved Kerr rotation technique is employed to study spin relaxation in Fe/MgO/GaAs heterostructures. The results reveal rich interactions between the GaAs electron spins, nuclear spins, and the
Dynamics of ferromagnetic spin glass: randomly canted ferromagnet versus skewed spin glass
NASA Astrophysics Data System (ADS)
Janutka, Andrzej
2003-12-01
A ferromagnetic spin glass (FSG) is one of the three isotropic and homogeneous phases of the long-range partially ordered magnets with spin and atomic disorder which are selected by symmetry (Andreev 1978 Sov. Phys.—JETP 47 411) (the others are genuine and antiferromagnetic spin glasses). The linear dynamical response to a magnetic field of two sub-phases of a FSG with drastically different dynamics, a randomly canted ferromagnet, in which the component spins create an acute angle with the summary magnetic moment, and a less-ordered skewed spin glass is analysed in the spin-wave approximation in the framework of phenomenological theory. The spin-wave damping coefficients and frequency shifts due to a magnon-magnon interaction are evaluated as functions of temperature and wavevector as well as the spectral-weight functions of the linear response to a magnetic field and the neutron scattering cross section which provides the possibility for experimental verification of the results. Substantial differences in the spin-wave characteristics of the FSG compared to those of the Heisenberg spin glass and the Heisenberg ferromagnet are found to be due to non-linear anisotropy effects in a FSG.
Dynamic control of spin wave spectra using spin-polarized currents
Wang, Qi; Zhang, Huaiwu Tang, Xiaoli; Bai, Feiming; Zhong, Zhiyong; Fangohr, Hans
2014-09-15
We describe a method of controlling the spin wave spectra dynamically in a uniform nanostripe waveguide through spin-polarized currents. A stable periodic magnetization structure is observed when the current flows vertically through the center of nanostripe waveguide. After being excited, the spin wave is transmitted at the sides of the waveguide. Numerical simulations of spin-wave transmission and dispersion curves reveal a single, pronounced band gap. Moreover, the periodic magnetization structure can be turned on and off by the spin-polarized current. The switching process from full rejection to full transmission takes place within less than 3 ns. Thus, this type magnonic waveguide can be utilized for low-dissipation spin wave based filters.
Shapiro like steps reveals molecular nanomagnets' spin dynamics
NASA Astrophysics Data System (ADS)
Abdollahipour, Babak; Abouie, Jahanfar; Ebrahimi, Navid
2015-09-01
We present an accurate way to detect spin dynamics of a nutating molecular nanomagnet by inserting it in a tunnel Josephson junction and studying the current voltage (I-V) characteristic. The spin nutation of the molecular nanomagnet is generated by applying two circularly polarized magnetic fields. We demonstrate that modulation of the Josephson current by the nutation of the molecular nanomagnet's spin appears as a stepwise structure like Shapiro steps in the I-V characteristic of the junction. Width and heights of these Shapiro-like steps are determined by two parameters of the spin nutation, frequency and amplitude of the nutation, which are simply tuned by the applied magnetic fields.
Gilbert damping of ferromagnetic metals incorporating inhomogeneous spin dynamics
Umetsu, Nobuyuki Miura, Daisuke; Sakuma, Akimasa
2015-05-07
The effects of inhomogeneous spin dynamics on magnetic damping in ferromagnetic metals are studied. On the basis of linear response theory, we derive the microscopic expression for the Gilbert damping term in a two-dimensional electron gas interacting with the magnetization via exchange coupling in the presence of Rashba spin-orbit coupling (SOC). In the spin wave propagating with the wave vector, q, the behavior of q-dependent damping can be explained in terms of both inter- and intra-band spin excitations. The spatially dependent damping torques originating from Rashba SOC that cancel out in a uniform precession system distort the circular orbit of a magnetization-precession trajectory in the presence of inhomogeneous spin dynamics.
Coherent Spin Dynamics in Semiconductor Nanostructures
NASA Astrophysics Data System (ADS)
Flatté, Michael E.
2004-03-01
Manipulation of coherent spins in semiconductors without laboratory AC (or in some cases DC) magnetic fields can be driven with the electronic spin-orbit interaction. This relativistic effect produces ``pseudomagnetic'' fields surpassing plausible laboratory magnetic fields by orders of magnitude. The theory of two principal examples will be described here: the coupling between light fields and electron spin in quantum dots, and the use of DC electric fields to manipulate spin coherence times in quantum wells. We find that intense coherent optical illumination of quantum dots can generate ultrafast ˜ 1000 Tesla pseudomagnetic fields suitable for electron spin rotation. These effective fields are roughly spherically symmetric for colloidal quantum dots, but for structurally aspherical quantum dots (such as self-assembled dots during molecular beam epitaxy growth) these pseudomagnetic fields are highly anisotropic - large parallel to the growth direction and often a factor of five or ten smaller along perpendicular directions. The structural anisotropy also leads to very anisotropic selection rules for light emission in quantum dot spin-light-emitting-diodes. For the second principal example, manipulation of spin coherence times in quantum wells, the zero-field spin coherence times and the tuning ranges depend strongly on the crystalline orientation of the growth axis. Near room temperature in (110)-grown structures for applied electric fields of 10-100 kV/cm, the tuning range can exceed several orders of magnitude. This work was done in collaboration with W. H. Lau and C. E. Pryor and was supported by DARPA/ARO and an ARO MURI.
Aging dynamics of quantum spin glasses of rotors
NASA Astrophysics Data System (ADS)
Kennett, Malcolm P.; Chamon, Claudio; Ye, Jinwu
2001-12-01
We study the long time dynamics of quantum spin glasses of rotors using the nonequilibrium Schwinger-Keldysh formalism. These models are known to have a quantum phase transition from a paramagnetic to a spin-glass phase, which we approach by looking at the divergence of the spin-relaxation rate at the transition point. In the aging regime, we determine the dynamical equations governing the time evolution of the spin response and correlation functions, and show that all terms in the equations that arise solely from quantum effects are irrelevant at long times under time reparametrization group (RPG) transformations. At long times, quantum effects enter only through the renormalization of the parameters in the dynamical equations for the classical counterpart of the rotor model. Consequently, quantum effects only modify the out-of-equilibrium fluctuation-dissipation relation (OEFDR), i.e. the ratio X between the temperature and the effective temperature, but not the form of the classical OEFDR.
Nonadiabatic multichannel dynamics of a spin-orbit-coupled condensate
NASA Astrophysics Data System (ADS)
Xiong, Bo; Zheng, Jun-hui; Wang, Daw-wei
2015-06-01
We investigate the nonadiabatic dynamics of a driven spin-orbit-coupled Bose-Einstein condensate in both weak and strong driven force. It is shown that the standard Landau-Zener (LZ) tunneling fails in the regime of weak driven force and/or strong spin-orbital coupling, where the full nonadiabatic dynamics requires a new mechanism through multichannel effects. Beyond the semiclassical approach, our numerical and analytical results show an oscillating power-law decay in the quantum limit, different from the exponential decay in the semiclassical limit of the LZ effect. Furthermore, the condensate density profile is found to be dynamically fragmented by the multichannel effects and enhanced by interaction effects. Our work therefore provides a complete picture to understand the nonadiabatic dynamics of a spin-orbit coupled condensate, including various ranges of driven force and interaction effects through multichannel interference. The experimental indication of these nonadiabatic dynamics is also discussed.
Vícha, Jan; Foroutan-Nejad, Cina; Pawlak, Tomasz; Munzarová, Markéta L; Straka, Michal; Marek, Radek
2015-04-14
The significant role of relativistic effects in altering the NMR chemical shifts of light nuclei in heavy-element compounds has been recognized for a long time; however, full understanding of this phenomenon in relation to the electronic structure has not been achieved. In this study, the recently observed qualitative differences between the platinum and gold compounds in the magnitude and the sign of spin-orbit-induced (SO) nuclear magnetic shielding at the vicinal light atom ((13)C, (15)N), σ(SO)(LA), are explained by the contractions of 6s and 6p atomic orbitals in Au complexes, originating in the larger Au nuclear charge and stronger scalar relativistic effects in gold complexes. This leads to the chemical activation of metal 6s and 6p atomic orbitals in Au complexes and their larger participation in bonding with the ligand, which modulates the propagation of metal-induced SO effects on the NMR signal of the LA via the Spin-Orbit/Fermi Contact (SO/FC) mechanism. The magnitude of the σ(SO)(LA) in these square-planar complexes can be understood on the basis of a balance between various metal-based 5d → 5d* and 6p → 6p* orbital magnetic couplings. The large and positive σ(SO)(LA) in platinum complexes is dominated by the shielding platinum-based 5d → 5d* magnetic couplings, whereas small or negative σ(SO)(LA) in gold complexes is related to the deshielding contribution of the gold-based 6p → 6p* magnetic couplings. Further, it is demonstrated that σ(SO)(LA) correlates quantitatively with the extent of M-LA electron sharing that is the covalence of the M-LA bond (characterized by the QTAIM delocalization index, DI). The present findings will contribute to further understanding of the origin and propagation of the relativistic effects influencing the experimental NMR parameters in heavy-element systems. PMID:26574362
Simulating spin dynamics in organic solids under heteronuclear decoupling.
Frantsuzov, Ilya; Ernst, Matthias; Brown, Steven P; Hodgkinson, Paul
2015-09-01
Although considerable progress has been made in simulating the dynamics of multiple coupled nuclear spins, predicting the evolution of nuclear magnetisation in the presence of radio-frequency decoupling remains challenging. We use exact numerical simulations of the spin dynamics under simultaneous magic-angle spinning and RF decoupling to determine the extent to which numerical simulations can be used to predict the experimental performance of heteronuclear decoupling for the CW, TPPM and XiX sequences, using the methylene group of glycine as a model system. The signal decay times are shown to be strongly dependent on the largest spin order simulated. Unexpectedly large differences are observed between the dynamics with and without spin echoes. Qualitative trends are well reproduced by modestly sized spin system simulations, and the effects of finite spin-system size can, in favourable cases, be mitigated by extrapolation. Quantitative prediction of the behaviour in complex parameter spaces is found, however, to be very challenging, suggesting that there are significant limits to the role of numerical simulations in RF decoupling problems, even when specialist techniques, such as state-space restriction, are used. PMID:26073419
The spin-temperature theory of dynamic nuclear polarization and nuclear spin-lattice relaxation
NASA Technical Reports Server (NTRS)
Byvik, C. E.; Wollan, D. S.
1974-01-01
A detailed derivation of the equations governing dynamic nuclear polarization (DNP) and nuclear spin lattice relaxation by use of the spin temperature theory has been carried to second order in a perturbation expansion of the density matrix. Nuclear spin diffusion in the rapid diffusion limit and the effects of the coupling of the electron dipole-dipole reservoir (EDDR) with the nuclear spins are incorporated. The complete expression for the dynamic nuclear polarization has been derived and then examined in detail for the limit of well resolved solid effect transitions. Exactly at the solid effect transition peaks, the conventional solid-effect DNP results are obtained, but with EDDR effects on the nuclear relaxation and DNP leakage factor included. Explicit EDDR contributions to DNP are discussed, and a new DNP effect is predicted.
Incomplete fusion dynamics by spin distribution measurements
Singh, D.; Ali, R.; Ansari, M. Afzal; Singh, Pushpendra P.; Sharma, M. K.; Singh, B. P.; Babu, K. Surendra; Sinha, Rishi K.; Kumar, R.; Muralithar, S.; Singh, R. P.; Bhowmik, R. K.
2010-02-15
Spin distributions for various evaporation residues populated via complete and incomplete fusion of {sup 16}O with {sup 124}Sn at 6.3 MeV/nucleon have been measured, using charged particles (Z=1,2)-{gamma} coincidence technique. Experimentally measured spin distributions of the residues produced as incomplete fusion products associated with 'fast'{alpha}- and 2{alpha}-emission channels observed in the 'forward cone' are found to be distinctly different from those of the residues produced as complete fusion products. Moreover, 'fast'{alpha}-particles that arise from larger angular momentum in the entrance channel are populated at relatively higher driving input angular momentum than those produced through complete fusion. The incomplete fusion residues are populated in a limited, higher-angular-momentum range, in contrast to the complete fusion products, which are populated over a broad spin range.
Universal Coarsening Dynamics of a Quenched Ferromagnetic Spin-1 Condensate
NASA Astrophysics Data System (ADS)
Williamson, Lewis A.; Blakie, P. B.
2016-01-01
We demonstrate that a quasi-two-dimensional spin-1 condensate quenched to a ferromagnetic phase undergoes universal coarsening in its late time dynamics. The quench can be implemented by a sudden change in the applied magnetic field and, depending on the final value, the ferromagnetic phase has easy-axis (Ising) or easy-plane (X Y ) symmetry, with different dynamical critical exponents. Our results for the easy-plane phase reveal a fractal domain structure and the crucial role of polar-core spin vortices in the coarsening dynamics.
Charge dynamics and spin order in doped Hubbard models
Kampf, A.P.; Brenig, W.
1994-04-01
Hole motion in an antiferromagnetic (AF) environment is accompanied by the emission of spin wave excitations. Spin-wave shakeoffs are responsible for incoherent contributions to the dynamics of propagating holes. Using a spin-density-wave polaron scheme the authors calculate the optical conductivity {sigma}({omega}) and show that the incoherent part of the hole spectrum contributes to the low-frequency part of {sigma}({omega}). Separately, the authors discuss the possible formation of spiral spin patterns upon doping of the half-filled one-band Hubbard model. In particular, the authors consider the influence of band structure effects arising from nearest- and next-nearest-neighbor hopping processes on a square lattice. Differences in the ground state spin patterns for hole and electron doping are obtained offering a possible explanation for the persistence of AF order in low electron-doped cuprate superconductors.
Ning Boyuan; Zhuang Jun; Zhang Wenxian; You, J. Q.
2011-07-15
We study the enhancement of spin coherence with periodic, concatenated, or Uhrig dynamical decoupling N-pulse sequences in a spin-1 Bose-Einstein condensate, where the intrinsic dynamical instability in such a ferromagnetically interacting condensate causes spin decoherence and eventually leads to a multiple spatial-domain structure or a spin texture. Our results show that all three sequences successfully enhance the spin coherence by pushing the wave vector of the most unstable mode in the condensate to a larger value. Among the three sequences with the same number of pulses, the concatenated one shows the best performance in preserving the spin coherence. More interestingly, we find that all three sequences exactly follow the same enhancement law, k{sub -}T{sup 1/2}=c, with k{sub -} the wave vector of the most unstable mode, T the sequence period, and c a sequence-dependent constant. Such a law between k{sub -} and T is also derived analytically for an attractive scalar Bose-Einstein condensate subjected to a periodic dynamical decoupling sequence.
Number Fluctuation Dynamics of Atomic Spin Mixing inside a Condensate
Chang, Lee; Zhai, Q.; Lu Rong; You, L.
2007-08-24
We investigate the quantum dynamics of number fluctuations inside an atomic condensate during coherent spin mixing among internal states of the ground state hyperfine manifold, by quantizing the semiclassical nonrigid pendulum model in terms of the conjugate variable pair: the relative phase and the atom number. Our result provides a theoretical basis that resolves the resolution limit, or the effective ''shot-noise'' level, for counting atoms that is needed to clearly detect quantum correlation effects in spin mixing.
Quantum Parallelism as a Tool for Ensemble Spin Dynamics Calculations
NASA Astrophysics Data System (ADS)
Álvarez, Gonzalo A.; Danieli, Ernesto P.; Levstein, Patricia R.; Pastawski, Horacio M.
2008-09-01
Efficient simulations of quantum evolutions of spin-1/2 systems are relevant for ensemble quantum computation as well as in typical NMR experiments. We propose an efficient method to calculate the dynamics of an observable provided that the initial excitation is “local.” It resorts to a single entangled pure initial state built as a superposition, with random phases, of the pure elements that compose the mixture. This ensures self-averaging of any observable, drastically reducing the calculation time. The procedure is tested for two representative systems: a spin star (cluster with random long range interactions) and a spin ladder.
Robust dynamical decoupling sequences for individual-nuclear-spin addressing
NASA Astrophysics Data System (ADS)
Casanova, J.; Wang, Z.-Y.; Haase, J. F.; Plenio, M. B.
2015-10-01
We propose the use of non-equally-spaced decoupling pulses for high-resolution selective addressing of nuclear spins by a quantum sensor. The analytical model of the basic operating principle is supplemented by detailed numerical studies that demonstrate the high degree of selectivity and the robustness against static and dynamic control-field errors of this scheme. We exemplify our protocol with a nitrogen-vacancy-center-based sensor to demonstrate that it enables the identification of individual nuclear spins that form part of a large spin ensemble.
Optically induced dynamic nuclear spin polarisation in diamond
NASA Astrophysics Data System (ADS)
Scheuer, Jochen; Schwartz, Ilai; Chen, Qiong; Schulze-Sünninghausen, David; Carl, Patrick; Höfer, Peter; Retzker, Alexander; Sumiya, Hitoshi; Isoya, Junichi; Luy, Burkhard; Plenio, Martin B.; Naydenov, Boris; Jelezko, Fedor
2016-01-01
The sensitivity of magnetic resonance imaging (MRI) depends strongly on nuclear spin polarisation and, motivated by this observation, dynamical nuclear spin polarisation has recently been applied to enhance MRI protocols (Kurhanewicz et al 2011 Neoplasia 13 81). Nuclear spins associated with the 13C carbon isotope (nuclear spin I = 1/2) in diamond possess uniquely long spin lattice relaxation times (Reynhardt and High 2011 Prog. Nucl. Magn. Reson. Spectrosc. 38 37). If they are present in diamond nanocrystals, especially when strongly polarised, they form a promising contrast agent for MRI. Current schemes for achieving nuclear polarisation, however, require cryogenic temperatures. Here we demonstrate an efficient scheme that realises optically induced 13C nuclear spin hyperpolarisation in diamond at room temperature and low ambient magnetic field. Optical pumping of a nitrogen-vacancy centre creates a continuously renewable electron spin polarisation which can be transferred to surrounding 13C nuclear spins. Importantly for future applications we also realise polarisation protocols that are robust against an unknown misalignment between magnetic field and crystal axis.
Theory of quantum control of spin-photon dynamics and spin decoherence in semiconductors
NASA Astrophysics Data System (ADS)
Yao, Wang
Single electron spin in a semiconductor quantum dot (QD) and single photon wavepacket propagating in an optical waveguide are investigated as carriers of quantum bit (qubit) for information processing. Cavity quantum electrodynamics of the coupled system composed of charged QD, microcavity and waveguide provides a quantum interface for the interplay of stationary spin qubits and flying photon qubits via cavity assisted optical control. This interface forms the basis for a wide range of essential functions of a quantum network, including transferring, swapping, and entangling qubits at distributed quantum nodes as well as a deterministic source and an efficient detector of a single photon wavepacket with arbitrarily specified shape. The cavity assisted optical process also made possible ultrafast initialization and QND readout of the spin qubit in QD. In addition, the strong optical nonlinearity of dot-cavity-waveguide coupled system enables phase gate and entanglement operation for flying single photon qubits in waveguides. The coherence of the electron spin is the wellspring of these quantum applications being investigated. At low temperature and strong magnetic field, the dominant cause of electron spin decoherence is the coupling with the interacting lattice nuclear spins. We present a quantum solution to the coupled dynamics of the electron with the nuclear spin bath. The decoherence is treated in terms of quantum entanglement of the electron with the nuclear pair-flip excitations driven by the various nuclear interactions. A novel nuclear interaction, mediated by virtue spin-flips of the single electron, plays an important role in single spin free-induction decay (FID). The spin echo not only refocuses the dephasing by inhomogeneous broadening in ensemble dynamics but also eliminates the decoherence by electron-mediated nuclear interaction. Thus, the decoherence times for single spin FID and ensemble spin echo are significantly different. The quantum theory of
Current-Induced Dynamics in Antiferromagnetic Metal: Domain Wall Dynamics and Spin Wave Excitation
NASA Astrophysics Data System (ADS)
Cheng, Ran; Niu, Qian
2013-03-01
When a spin-polarized current flows through a ferromagnetic (FM) metal, angular momentum is transferred to the magnetization via spin transfer torque. However, corresponding theory is absent in antiferromagnetic (AFM) metals due to the absence of spin conservation. We solve this problem via effective gauge theory without the necessity of spin conservation. By identifying the adiabatic dynamics of conduction electrons as a non-Abelian gauge theory on degenerate band, we derive the AFM version of Landau-Lifshitz-Gilbert equation with current-induced dynamics from a microscopic point of view. Quite different from its FM counterpart, current-induced dynamics in AFM materials does not behave as a torque, but a driving force triggering second order derivative of local staggered order with respect to time. Its physical consequences are studied in two examples: 1. A domain wall is accelerated to a terminal velocity without a Walker's threshold; 2. A sufficiently large spin current will generate spin wave excitation.
Storing entanglement of nuclear spins via Uhrig dynamical decoupling
Roy, Soumya Singha; Mahesh, T. S.; Agarwal, G. S.
2011-06-15
Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single-qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal order of the Uhrig sequence in which a singlet state can be stored at high correlation for about 30 seconds.
Dynamics and hysteresis in square lattice artificial spin ice
NASA Astrophysics Data System (ADS)
Wysin, G. M.; Moura-Melo, W. A.; Mól, L. A. S.; Pereira, A. R.
2013-04-01
Dynamical effects under geometrical frustration are considered in a model for artificial spin ice on a square lattice in two dimensions. Each island of the spin ice has a three-component Heisenberg-like dipole moment subject to shape anisotropies that influence its direction. The model has real dynamics, including rotation of the magnetic degrees of freedom, going beyond the Ising-type models of spin ice. The dynamics is studied using a Langevin equation solved via a second-order Heun algorithm. Thermodynamic properties such as the specific heat are presented for different couplings. A peak in specific heat is related to a type of melting-like phase transition present in the model. Hysteresis in an applied magnetic field is calculated for model parameters where the system is able to reach thermodynamic equilibrium.
Spin-orbital dynamics in a system of polar molecules
NASA Astrophysics Data System (ADS)
Syzranov, Sergey; Wall, Michael; Gurarie, Victor; Rey, Ana Maria
2015-05-01
We consider the dynamics of a two-dimensional system of ultracold polar molecules weakly perturbed from a stationary state. We demonstrate that dipole-dipole interactions in such a system generate chiral excitations with a non-trivial Berry phase 2 π . These excitations, which we call chirons, resemble low-energy quasiparticles in bilayer graphene and emerge regardless of the quantum statistics and for arbitrary ratios of kinetic to interaction energies. Chirons manifest themselves in the dynamics of the spin density profile, spin currents, and spin coherences, even for molecules pinned in a deep optical lattice. We derive the kinetic equation that describes chiron dynamics and calculate the distributions of physical observables for experimentally realisable initial conditions. This work was supported by NIST: JILA-NSF-PFC-1125844, NSF-PIF-1211914, NSF-PHY11-25915, ARO, ARO-DARPA-OLE, AFOSR, AFOSR-MURI; NSF: DMR-1001240, PHY-1125844, and the Alexander von Humboldt Foundation.
Dynamics of magnetization in ferromagnet with spin-transfer torque
NASA Astrophysics Data System (ADS)
Li, Zai-Dong; He, Peng-Bin; Liu, Wu-Ming
2014-11-01
We review our recent works on dynamics of magnetization in ferromagnet with spin-transfer torque. Driven by constant spin-polarized current, the spin-transfer torque counteracts both the precession driven by the effective field and the Gilbert damping term different from the common understanding. When the spin current exceeds the critical value, the conjunctive action of Gilbert damping and spin-transfer torque leads naturally the novel screw-pitch effect characterized by the temporal oscillation of domain wall velocity and width. Driven by space- and time-dependent spin-polarized current and magnetic field, we expatiate the formation of domain wall velocity in ferromagnetic nanowire. We discuss the properties of dynamic magnetic soliton in uniaxial anisotropic ferromagnetic nanowire driven by spin-transfer torque, and analyze the modulation instability and dark soliton on the spin wave background, which shows the characteristic breather behavior of the soliton as it propagates along the ferromagnetic nanowire. With stronger breather character, we get the novel magnetic rogue wave and clarify its formation mechanism. The generation of magnetic rogue wave mainly arises from the accumulation of energy and magnons toward to its central part. We also observe that the spin-polarized current can control the exchange rate of magnons between the envelope soliton and the background, and the critical current condition is obtained analytically. At last, we have theoretically investigated the current-excited and frequency-adjusted ferromagnetic resonance in magnetic trilayers. A particular case of the perpendicular analyzer reveals that the ferromagnetic resonance curves, including the resonant location and the resonant linewidth, can be adjusted by changing the pinned magnetization direction and the direct current. Under the control of the current and external magnetic field, several magnetic states, such as quasi-parallel and quasi-antiparallel stable states, out
Tunable nonequilibrium dynamics of field quenches in spin ice
Mostame, Sarah; Castelnovo, Claudio; Moessner, Roderich; Sondhi, Shivaji L.
2014-01-01
We present nonequilibrium physics in spin ice as a unique setting that combines kinematic constraints, emergent topological defects, and magnetic long-range Coulomb interactions. In spin ice, magnetic frustration leads to highly degenerate yet locally constrained ground states. Together, they form a highly unusual magnetic state—a “Coulomb phase”—whose excitations are point-like defects—magnetic monopoles—in the absence of which effectively no dynamics is possible. Hence, when they are sparse at low temperature, dynamics becomes very sluggish. When quenching the system from a monopole-rich to a monopole-poor state, a wealth of dynamical phenomena occur, the exposition of which is the subject of this article. Most notably, we find reaction diffusion behavior, slow dynamics owing to kinematic constraints, as well as a regime corresponding to the deposition of interacting dimers on a honeycomb lattice. We also identify potential avenues for detecting the magnetic monopoles in a regime of slow-moving monopoles. The interest in this model system is further enhanced by its large degree of tunability and the ease of probing it in experiment: With varying magnetic fields at different temperatures, geometric properties—including even the effective dimensionality of the system—can be varied. By monitoring magnetization, spin correlations or zero-field NMR, the dynamical properties of the system can be extracted in considerable detail. This establishes spin ice as a laboratory of choice for the study of tunable, slow dynamics. PMID:24379372
Dynamics of a mesoscopic nuclear spin ensemble interacting with an optically driven electron spin
NASA Astrophysics Data System (ADS)
Stanley, M. J.; Matthiesen, C.; Hansom, J.; Le Gall, C.; Schulte, C. H. H.; Clarke, E.; Atatüre, M.
2014-11-01
The ability to discriminate between simultaneously occurring noise sources in the local environment of semiconductor InGaAs quantum dots, such as electric and magnetic field fluctuations, is key to understanding their respective dynamics and their effect on quantum dot coherence properties. We present a discriminatory approach to all-optical sensing based on two-color resonance fluorescence of a quantum dot charged with a single electron. Our measurements show that local magnetic field fluctuations due to nuclear spins in the absence of an external magnetic field are described by two correlation times, both in the microsecond regime. The nuclear spin bath dynamics show a strong dependence on the strength of resonant probing, with correlation times increasing by a factor of 4 as the optical transition is saturated. We interpret the behavior as motional averaging of both the Knight field of the resident electron spin and the hyperfine-mediated nuclear spin-spin interaction due to optically induced electron spin flips.
Theoretical aspects of Magic Angle Spinning - Dynamic Nuclear Polarization
NASA Astrophysics Data System (ADS)
Mentink-Vigier, Frederic; Akbey, Ümit; Oschkinat, Hartmut; Vega, Shimon; Feintuch, Akiva
2015-09-01
Magic Angle Spinning (MAS) combined with Dynamic Nuclear Polarization (DNP) has been proven in recent years to be a very powerful method for increasing solid-state NMR signals. Since the advent of biradicals such as TOTAPOL to increase the nuclear polarization new classes of radicals, with larger molecular weight and/or different spin properties have been developed. These have led to unprecedented signal gain, with varying results for different experimental parameters, in particular the microwave irradiation strength, the static field, and the spinning frequency. Recently it has been demonstrated that sample spinning imposes DNP enhancement processes that differ from the active DNP mechanism in static samples as upon sample spinning the DNP enhancements are the results of energy level anticrossings occurring periodically during each rotor cycle. In this work we present experimental results with regards to the MAS frequency dependence of the DNP enhancement profiles of four nitroxide-based radicals at two different sets of temperature, 110 and 160 K. In fact, different magnitudes of reduction in enhancement are observed with increasing spinning frequency. Our simulation code for calculating MAS-DNP powder enhancements of small model spin systems has been improved to extend our studies of the influence of the interaction and relaxation parameters on powder enhancements. To achieve a better understanding we simulated the spin dynamics of a single three-spin system {ea -eb - n } during its steady state rotor periods and used the Landau-Zener formula to characterize the influence of the different anti-crossings on the polarizations of the system and their necessary action for reaching steady state conditions together with spin relaxation processes. Based on these model calculations we demonstrate that the maximum steady state nuclear polarization cannot become larger than the maximum polarization difference between the two electrons during the steady state rotor cycle
Theoretical aspects of Magic Angle Spinning - Dynamic Nuclear Polarization.
Mentink-Vigier, Frederic; Akbey, Ümit; Oschkinat, Hartmut; Vega, Shimon; Feintuch, Akiva
2015-09-01
Magic Angle Spinning (MAS) combined with Dynamic Nuclear Polarization (DNP) has been proven in recent years to be a very powerful method for increasing solid-state NMR signals. Since the advent of biradicals such as TOTAPOL to increase the nuclear polarization new classes of radicals, with larger molecular weight and/or different spin properties have been developed. These have led to unprecedented signal gain, with varying results for different experimental parameters, in particular the microwave irradiation strength, the static field, and the spinning frequency. Recently it has been demonstrated that sample spinning imposes DNP enhancement processes that differ from the active DNP mechanism in static samples as upon sample spinning the DNP enhancements are the results of energy level anticrossings occurring periodically during each rotor cycle. In this work we present experimental results with regards to the MAS frequency dependence of the DNP enhancement profiles of four nitroxide-based radicals at two different sets of temperature, 110 and 160K. In fact, different magnitudes of reduction in enhancement are observed with increasing spinning frequency. Our simulation code for calculating MAS-DNP powder enhancements of small model spin systems has been improved to extend our studies of the influence of the interaction and relaxation parameters on powder enhancements. To achieve a better understanding we simulated the spin dynamics of a single three-spin system {ea-eb-n} during its steady state rotor periods and used the Landau-Zener formula to characterize the influence of the different anti-crossings on the polarizations of the system and their necessary action for reaching steady state conditions together with spin relaxation processes. Based on these model calculations we demonstrate that the maximum steady state nuclear polarization cannot become larger than the maximum polarization difference between the two electrons during the steady state rotor cycle. This
Dynamics of a spinning particle in a linear in spin Hamiltonian approximation
NASA Astrophysics Data System (ADS)
Lukes-Gerakopoulos, Georgios; Katsanikas, Matthaios; Patsis, Panos A.; Seyrich, Jonathan
2016-07-01
We investigate for order and chaos the dynamical system of a spinning test particle of mass m moving in the spacetime background of a Kerr black hole of mass M . This system is approximated in our investigation by the linear in spin Hamiltonian function [E. Barausse and A. Buonanno, Phys. Rev. D 81, 084024 (2010)]. We study the corresponding phase space by using 2D projections on a surface of section and the method of color and rotation on a 4D Poincaré section. Various topological structures coming from the nonintegrability of the linear in spin Hamiltonian are found and discussed. Moreover, an interesting result is that from the value of the dimensionless spin S /(m M )=10-4 of the particle and below, the impact of the nonintegrability of the system on the motion of the particle seems to be negligible.
Quench dynamics and relaxation in isolated integrable quantum spin chains
NASA Astrophysics Data System (ADS)
Essler, Fabian H. L.; Fagotti, Maurizio
2016-06-01
We review the dynamics after quantum quenches in integrable quantum spin chains. We give a pedagogical introduction to relaxation in isolated quantum systems, and discuss the description of the steady state by (generalized) Gibbs ensembles. We then turn to general features in the time evolution of local observables after the quench, using a simple model of free fermions as an example. In the second part we present an overview of recent progress in describing quench dynamics in two key paradigms for quantum integrable models, the transverse field Ising chain and the anisotropic spin-1/2 Heisenberg chain.
Destination state screening of active spaces in spin dynamics simulations
NASA Astrophysics Data System (ADS)
Krzystyniak, M.; Edwards, Luke J.; Kuprov, Ilya
2011-06-01
We propose a novel avenue for state space reduction in time domain Liouville space spin dynamics simulations, using detectability as a selection criterion - only those states that evolve into or affect other detectable states are kept in the simulation. This basis reduction procedure (referred to as destination state screening) is formally exact and can be applied on top of the existing state space restriction techniques. As demonstrated below, in many cases this results in further reduction of matrix dimension, leading to considerable acceleration of many spin dynamics simulation types. Destination state screening is implemented in the latest version of the Spinach library (http://spindynamics.org).
Local spin dynamics with the electron electric dipole moment
NASA Astrophysics Data System (ADS)
Fukuda, Masahiro; Soga, Kota; Senami, Masato; Tachibana, Akitomo
2016-01-01
The local spin dynamics of the electron is studied from the viewpoint of the electric dipole moment (EDM) of the electron in the framework of the quantum field theory. The improvements of the computational accuracy of the effective electric field (Eeff) for the EDM and the understanding of spin precession are important for the experimental determination of the upper bound of the EDM. Calculations of Eeff in YbF (2Σ1 /2 ), BaF (2Σ1 /2 ), ThO (3Δ1 ), and HF+ (2Π1 /2 ) are performed on the basis of the restricted active space configuration interaction approach by using the four-component relativistic electronic structure calculation. The spin precession is also discussed from the viewpoint of local spin torque dynamics. We show that a contribution to the torque density for the spin is brought into by the EDM. Distributions of the local spin angular momentum density and torque densities induced by external fields in the above molecules are calculated and a property related with large Eeff is discussed.
Hole dynamics in spin and orbital ordered vanadium perovskites
NASA Astrophysics Data System (ADS)
Ishihara, Sumio
2005-03-01
We present a theory of the doped perovskite vanadates with spin and orbital orders [1]. Two kinds of spin-orbital orders are found in the ground state: the G-type (three-dimensional (3D) staggered) spin order (SO) with the C-type (rod type) orbital order (OO) (the alternative dxy^1dyz^1/dxy^1dzx^1 configuration) termed (SG/OC) in YVO3, and the C-type SO with the G-type OO termed (SC/OG) in LaVO3. Mobile holes are strongly renormalized by spin excitations (magnons) in the spin G-type and orbital C-type (SG/OC) order, and orbital excitations (orbitons) in the spin C-type and orbital G-type (SC/OG) one. It is found that hole dynamics in a staggered t2g orbital array is distinct from that in a antiferromagnetic order as well as the eg orbital one. The anomalously fragile character of the (SG/OC) order observed in Y1-xCaxVO3 is attributed to the orbiton softening induced by a reduction of the spin order parameter. [1] S. Ishihara, cond-mat/0408395.
Shapiro like steps reveals molecular nanomagnets’ spin dynamics
Abdollahipour, Babak; Abouie, Jahanfar Ebrahimi, Navid
2015-09-15
We present an accurate way to detect spin dynamics of a nutating molecular nanomagnet by inserting it in a tunnel Josephson junction and studying the current voltage (I-V) characteristic. The spin nutation of the molecular nanomagnet is generated by applying two circularly polarized magnetic fields. We demonstrate that modulation of the Josephson current by the nutation of the molecular nanomagnet’s spin appears as a stepwise structure like Shapiro steps in the I-V characteristic of the junction. Width and heights of these Shapiro-like steps are determined by two parameters of the spin nutation, frequency and amplitude of the nutation, which are simply tuned by the applied magnetic fields.
Protecting and enhancing spin squeezing via continuous dynamical decoupling
NASA Astrophysics Data System (ADS)
Chaudhry, Adam Zaman; Gong, Jiangbin
2012-07-01
Realizing useful quantum operations with high fidelity is a two-task quantum control problem wherein decoherence is to be suppressed and desired unitary evolution is to be executed. The dynamical decoupling (DD) approach to decoherence suppression has been fruitful but synthesizing DD fields with certain quantum control fields may be experimentally demanding. In the context of spin squeezing, here we explore an unforeseen possibility that continuous DD fields may serve dual purposes at once. In particular, it is shown that a rather simple configuration of DD fields can suppress collective decoherence and yield a 1/N scaling of the squeezing performance (N is the number of spins), thus making spin squeezing more robust to noise and much closer to the so-called Heisenberg limit. The theoretical predictions should be within the reach of current spin squeezing experiments.
Spin Dynamics during Ultrafast Optical Demagnetization
NASA Astrophysics Data System (ADS)
Eisebitt, Stefan
2015-03-01
Magnetic order can be influenced on a sub-picosecund time scale via femtosecond optical pulses. In particular, demagnetization and switching can be triggered optically and while the applications e.g. for magnetic data storage are obvious, the underlying mechanisms are still under debate. We have investigated the contribution of electronic transport to optical demagnetization via pump-probe experiments at free-electron x-ray lasers. In ferromagnetic thin film multilayers with perpendicular anisotropy, optically excited electrons can move within a labyrinth domain network. Using x-ray magnetic circular dichroism (XMCD) as a contrast mechanism for small angle x-ray scattering to probe the local magnetization, we observe an ultrafast broadening of the domain walls, consistent with the existence of superdiffusive spin currents. Via pump-probe x-ray holographic imaging we obtain real space images of the local magnetization within the domain structure after pumping the system by a laterally confined excitation generated by an optical standing wave. With a temporal resolution of about 100 fs, we observe the propagation of a demagnetization front in real space, again consistent with the existence of superdiffusive spin currents. Support by BMBF in FSP-301 and 302 via Contracts 05K10KTB, 05K13KT3 and 05K13KT4 is gratefully acknowledged.
Combined Molecular Dynamics-Spin Dynamics Simulation of α-Iron in an External Magnetic Field
NASA Astrophysics Data System (ADS)
Mudrick, Mark; Perera, Dilina; Landau, David P.
Using an atomistic model that treats both translational and spin degrees of freedom, combined molecular and spin dynamics simulations have been performed to study dynamic properties of α-iron. Atomic interactions are described by an empirical many-body potential while spin-spin interactions are handled with a Heisenberg-like Hamiltonian with a coordinate dependent exchange interaction. Each of these interactions are parameterized by first-principles calculations. These simulations numerically solve equations of motion using an algorithm based on the second-order Suzuki-Trotter decomposition for the time evolution operator. Through calculation of the Fourier transform of space-displaced time-displaced correlation functions, vibrational and magnetic excitations have been studied. The application of an external magnetic field up to 10-T has now been included and has been shown to increase the characteristic frequencies of the single-spin-wave excitations. Two-spin-wave interactions have also been investigated.
Investigations of quantum pendulum dynamics in a spin-1 BEC
NASA Astrophysics Data System (ADS)
Hoang, Thai; Gerving, Corey; Land, Ben; Anquez, Martin; Hamley, Chris; Chapman, Michael
2013-05-01
We investigate the quantum spin dynamics of a spin-1 BEC initialized to an unstable critical point of the dynamical phase space. The subsequent evolution of the collective states of the system is analogous to an inverted simple pendulum in the quantum limit and yields non-classical states with quantum correlations. For short evolution times in the low depletion limit, we observe squeezed states and for longer times beyond the low depletion limit we observe highly non-Gaussian distributions. C.D. Hamley, C.S. Gerving, T.M. Hoang, E.M. Bookjans, and M.S. Chapman, ``Spin-Nematic Squeezed Vacuum in a Quantum Gas,'' Nature Physics 8, 305-308 (2012).
Controlling the quantum dynamics of a mesoscopic spin bath in diamond
de Lange, Gijs; van der Sar, Toeno; Blok, Machiel; Wang, Zhi-Hui; Dobrovitski, Viatcheslav; Hanson, Ronald
2012-01-01
Understanding and mitigating decoherence is a key challenge for quantum science and technology. The main source of decoherence for solid-state spin systems is the uncontrolled spin bath environment. Here, we demonstrate quantum control of a mesoscopic spin bath in diamond at room temperature that is composed of electron spins of substitutional nitrogen impurities. The resulting spin bath dynamics are probed using a single nitrogen-vacancy (NV) centre electron spin as a magnetic field sensor. We exploit the spin bath control to dynamically suppress dephasing of the NV spin by the spin bath. Furthermore, by combining spin bath control with dynamical decoupling, we directly measure the coherence and temporal correlations of different groups of bath spins. These results uncover a new arena for fundamental studies on decoherence and enable novel avenues for spin-based magnetometry and quantum information processing. PMID:22536480
Magnetization dynamics of imprinted non-collinear spin textures
Streubel, Robert Kopte, Martin; Makarov, Denys; Fischer, Peter; Schmidt, Oliver G.
2015-09-14
We study the magnetization dynamics of non-collinear spin textures realized via imprint of the magnetic vortex state in soft permalloy into magnetically hard out-of-plane magnetized Co/Pd nanopatterned heterostructures. Tuning the interlayer exchange coupling between soft- and hard-magnetic subsystems provides means to tailor the magnetic state in the Co/Pd stack from being vortex- to donut-like with different core sizes. While the imprinted vortex spin texture leads to the dynamics similar to the one observed for vortices in permalloy disks, the donut-like state causes the appearance of two gyrofrequencies characteristic of the early and later stages of the magnetization dynamics. The dynamics are described using the Thiele equation supported by the full scale micromagnetic simulations by taking into account an enlarged core size of the donut states compared to magnetic vortices.
Spin dynamics of paramagnetic centers with anisotropic g tensor and spin of 1/2.
Maryasov, Alexander G; Bowman, Michael K
2012-08-01
The influence of g tensor anisotropy on spin dynamics of paramagnetic centers having real or effective spin of 1/2 is studied. The g anisotropy affects both the excitation and the detection of EPR signals, producing noticeable differences between conventional continuous-wave (cw) EPR and pulsed EPR spectra. The magnitudes and directions of the spin and magnetic moment vectors are generally not proportional to each other, but are related to each other through the g tensor. The equilibrium magnetic moment direction is generally parallel to neither the magnetic field nor the spin quantization axis due to the g anisotropy. After excitation with short microwave pulses, the spin vector precesses around its quantization axis, in a plane that is generally not perpendicular to the applied magnetic field. Paradoxically, the magnetic moment vector precesses around its equilibrium direction in a plane exactly perpendicular to the external magnetic field. In the general case, the oscillating part of the magnetic moment is elliptically polarized and the direction of precession is determined by the sign of the g tensor determinant (g tensor signature). Conventional pulsed and cw EPR spectrometers do not allow determination of the g tensor signature or the ellipticity of the magnetic moment trajectory. It is generally impossible to set a uniform spin turning angle for simple pulses in an unoriented or 'powder' sample when g tensor anisotropy is significant. PMID:22743542
SPIN DYNAMICS IN AGS AND RHIC.
Mackay, W W; Bai, M; Courant, E D; Brown, K; Glenn, W; Huang, H; Luccio, A; Ptitsyn, V; Roser, T; Satogata, T; Ltepikian, S; Tsoupas, N; Zelenski, A
2003-05-12
A fundamental aspect of particle physics is the spin of the particles. With polarized beams, the internal structure of the proton may be probed in ways that are unattainable with unpolarized beams. The Relativistic Heavy Ion Collider (RHIC) has the unique capability of colliding protons with both transverse and longitudinal polarization at center-of-mass energies up to 500 GeV. In this paper we examine the methods used to accelerate and manipulate polarized proton beams in RHIC and its injectors. Special techniques include the use of a partial Siberian snake and an ac dipole in the AGS. In RHIC we use four superconducting helical Siberian snakes (two per ring) for acceleration, and eight superconducting helical rotators for independent control of polarization directions at two interaction regions.
Dynamical spin-density waves in a spin-orbit-coupled Bose-Einstein condensate
NASA Astrophysics Data System (ADS)
Li, Yan; Qu, Chunlei; Zhang, Yongsheng; Zhang, Chuanwei
2015-07-01
Synthetic spin-orbit (SO) coupling, an important ingredient for quantum simulation of many exotic condensed matter physics, has recently attracted considerable attention. The static and dynamic properties of a SO-coupled Bose-Einstein condensate (BEC) have been extensively studied in both theory and experiment. Here we numerically investigate the generation and propagation of a dynamical spin-density wave (SDW) in a SO-coupled BEC using a fast moving Gaussian-shaped barrier. We find that the SDW wavelength is sensitive to the barrier's velocity while varies slightly with the barrier's peak potential or width. We qualitatively explain the generation of SDW by considering a rectangular barrier in a one-dimensional system. Our results may motivate future experimental and theoretical investigations of rich dynamics in the SO-coupled BEC induced by a moving barrier.
Spin and orbital exchange interactions from Dynamical Mean Field Theory
NASA Astrophysics Data System (ADS)
Secchi, A.; Lichtenstein, A. I.; Katsnelson, M. I.
2016-02-01
We derive a set of equations expressing the parameters of the magnetic interactions characterizing a strongly correlated electronic system in terms of single-electron Green's functions and self-energies. This allows to establish a mapping between the initial electronic system and a spin model including up to quadratic interactions between the effective spins, with a general interaction (exchange) tensor that accounts for anisotropic exchange, Dzyaloshinskii-Moriya interaction and other symmetric terms such as dipole-dipole interaction. We present the formulas in a format that can be used for computations via Dynamical Mean Field Theory algorithms.
Computer studies of multiple-quantum spin dynamics
Murdoch, J.B.
1982-11-01
The excitation and detection of multiple-quantum (MQ) transitions in Fourier transform NMR spectroscopy is an interesting problem in the quantum mechanical dynamics of spin systems as well as an important new technique for investigation of molecular structure. In particular, multiple-quantum spectroscopy can be used to simplify overly complex spectra or to separate the various interactions between a nucleus and its environment. The emphasis of this work is on computer simulation of spin-system evolution to better relate theory and experiment.
On the spin-axis dynamics of a Moonless Earth
Li, Gongjie; Batygin, Konstantin
2014-07-20
The variation of a planet's obliquity is influenced by the existence of satellites with a high mass ratio. For instance, Earth's obliquity is stabilized by the Moon and would undergo chaotic variations in the Moon's absence. In turn, such variations can lead to large-scale changes in the atmospheric circulation, rendering spin-axis dynamics a central issue for understanding climate. The relevant quantity for dynamically forced climate change is the rate of chaotic diffusion. Accordingly, here we re-examine the spin-axis evolution of a Moonless Earth within the context of a simplified perturbative framework. We present analytical estimates of the characteristic Lyapunov coefficient as well as the chaotic diffusion rate and demonstrate that even in absence of the Moon, the stochastic change in Earth's obliquity is sufficiently slow to not preclude long-term habitability. Our calculations are consistent with published numerical experiments and illustrate the putative system's underlying dynamical structure in a simple and intuitive manner.
Solvent effects and dynamic averaging of 195Pt NMR shielding in cisplatin derivatives.
Truflandier, Lionel A; Sutter, Kiplangat; Autschbach, Jochen
2011-03-01
The influences of solvent effects and dynamic averaging on the (195)Pt NMR shielding and chemical shifts of cisplatin and three cisplatin derivatives in aqueous solution were computed using explicit and implicit solvation models. Within the density functional theory framework, these simulations were carried out by combining ab initio molecular dynamics (aiMD) simulations for the phase space sampling with all-electron relativistic NMR shielding tensor calculations using the zeroth-order regular approximation. Structural analyses support the presence of a solvent-assisted "inverse" or "anionic" hydration previously observed in similar square-planar transition-metal complexes. Comparisons with computationally less demanding implicit solvent models show that error cancellation is ubiquitous when dealing with liquid-state NMR simulations. After aiMD averaging, the calculated chemical shifts for the four complexes are in good agreement with experiment, with relative deviations between theory and experiment of about 5% on average (1% of the Pt(II) chemical shift range). PMID:21204547
Dynamic-angle spinning and double rotation of quadrupolar nuclei
NASA Astrophysics Data System (ADS)
Mueller, K. T.
1991-07-01
Nuclear magnetic resonance (NMR) spectroscopy of quadrupolar nuclei is complicated by the coupling of the electric quadrupole moment of the nucleus to local variations in the electric field. The quadrupolar interaction is a useful source of information about local molecular structure in solids, but it tends to broaden resonance lines, causing crowding and overlap in NMR spectra. Magic-angle spinning, which is routinely used to produce high resolution spectra of spin-1/2 nuclei like carbon-13 and silicon-29, is incapable of fully narrowing resonances from quadrupolar nuclei when anisotropic second-order quadrupolar interactions are present. Two new sample-spinning techniques are introduced here that completely average the second-order quadrupolar coupling. Narrow resonance lines are obtained and individual resonances from distinct nuclear sites are identified. In dynamic-angle spinning (DAS) a rotor containing a powdered sample is reoriented between discrete angles with respect to high magnetic field. Evolution under anisotropic interactions at the different angles cancels, leaving only the isotropic evolution of the spin system. In the second technique, double rotation (DOR), a small rotor spins within a larger rotor so that the sample traces out a complicated trajectory in space. The relative orientation of the rotors and the orientation of the larger rotor within the magnetic field are selected to average both first- and second-order anisotropic broadening. The theory of quadrupolar interactions, coherent averaging theory, and motional narrowing by sample reorientation are reviewed with emphasis on the chemical shift anisotropy and second-order quadrupolar interactions experienced by half-odd integer spin quadrupolar nuclei. The DAS and DOR techniques are introduced and illustrated with application to common quadrupolar systems such as sodium-23 and oxygen-17 nuclei in solids.
Dynamic-angle spinning and double rotation of quadrupolar nuclei
Mueller, K.T. California Univ., Berkeley, CA . Dept. of Chemistry)
1991-07-01
Nuclear magnetic resonance (NMR) spectroscopy of quadrupolar nuclei is complicated by the coupling of the electric quadrupole moment of the nucleus to local variations in the electric field. The quadrupolar interaction is a useful source of information about local molecular structure in solids, but it tends to broaden resonance lines causing crowding and overlap in NMR spectra. Magic- angle spinning, which is routinely used to produce high resolution spectra of spin-{1/2} nuclei like carbon-13 and silicon-29, is incapable of fully narrowing resonances from quadrupolar nuclei when anisotropic second-order quadrupolar interactions are present. Two new sample-spinning techniques are introduced here that completely average the second-order quadrupolar coupling. Narrow resonance lines are obtained and individual resonances from distinct nuclear sites are identified. In dynamic-angle spinning (DAS) a rotor containing a powdered sample is reoriented between discrete angles with respect to high magnetic field. Evolution under anisotropic interactions at the different angles cancels, leaving only the isotropic evolution of the spin system. In the second technique, double rotation (DOR), a small rotor spins within a larger rotor so that the sample traces out a complicated trajectory in space. The relative orientation of the rotors and the orientation of the larger rotor within the magnetic field are selected to average both first- and second-order anisotropic broadening. The theory of quadrupolar interactions, coherent averaging theory, and motional narrowing by sample reorientation are reviewed with emphasis on the chemical shift anisotropy and second-order quadrupolar interactions experienced by half-odd integer spin quadrupolar nuclei. The DAS and DOR techniques are introduced and illustrated with application to common quadrupolar systems such as sodium-23 and oxygen-17 nuclei in solids.
Anisotropies and spin dynamics in ultrathin magnetic multilayer structures
NASA Astrophysics Data System (ADS)
Kardasz, Bartlomiej
High quality magnetic films were prepared by Molecular Beam Epitaxy (MBE) using Thermal Deposition (TD) and Pulse Laser Deposition (PLD) techniques. Ferromagnetic Resonance (FMR) and Mossbauer studies have shown that the Fe films prepared by PLD exhibited a more intermixed interface lattice structure than those prepared by TD. Dramatic decrease of the in-plane interface uniaxial anisotropy for the PLD films compared to those prepared by TD has shown that the in-plane uniaxial anisotropy is caused by magnetoelasticity driven by the Fe/GaAs(001) interface lattice shear. Magnetization dynamics of the ultrathin Fe/Au,Ag/Fe films was studied using Time-Resolved Magneto-Optical Kerr Effect (TRMOKE) and FMR in the frequency range from 1 to 73 GHz. The Gilbert damping was studied in the Au/Fe/GaAs(001) structures as a function of the Fe and Au layer thickness, respectively. The observed increase in magnetic damping in the Fe film covered with thick Au capping layers was explained by spin pumping at the Fe/Au interface accompanied by spin relaxation and diffusion of the accumulated spin density in the Au layer. The spin diffusion length in Au was found to be 34 nm at room temperature. Significant increase of the Gilbert damping was observed in the Au/Fe/GaAs structures with decreasing Fe film thickness. Its origin lies in the additional damping at the Fe/GaAs interface. Direct detection of the spin current propagating across the Ag spacer in Fe/Ag,Au/Fe/GaAs(001) structures was carried out with stroboscopic TRMOKE measurements. The Fe layer grown on GaAs served as a spin pumping source and the Fe layer grown on the Au,Ag spacer was used as a probe for detection of the spin current propagating across the Au and Ag spacers. The experimental results were interpreted using selfconsistent solution of the Landau Lifshitz Gilbert (LLG) equations of motion with the spin diffusion equation for the accumulated spin density in the Au and Ag spacers. The spin diffusion length in Ag was
Spacetime dynamics of spinning particles: Exact electromagnetic analogies
NASA Astrophysics Data System (ADS)
Costa, L. Filipe O.; Natário, José; Zilhão, Miguel
2016-05-01
We compare the rigorous equations describing the motion of spinning test particles in gravitational and electromagnetic fields, and show that if the Mathisson-Pirani spin condition holds then exact gravito-electromagnetic analogies emerge. These analogies provide a familiar formalism to treat gravitational problems, as well as a means for comparing the two interactions. Fundamental differences are manifest in the symmetries and time projections of the electromagnetic and gravitational tidal tensors. The physical consequences of the symmetries of the tidal tensors are explored comparing the following analogous setups: magnetic dipoles in the field of nonspinning/spinning charges, and gyroscopes in the Schwarzschild, Kerr, and Kerr-de Sitter spacetimes. The implications of the time projections of the tidal tensors are illustrated by the work done on the particle in various frames; in particular, a reciprocity is found to exist: in a frame comoving with the particle, the electromagnetic (but not the gravitational) field does work on it, causing a variation of its proper mass; conversely, for "static observers," a stationary gravitomagnetic (but not a magnetic) field does work on the particle, and the associated potential energy is seen to embody the Hawking-Wald spin-spin interaction energy. The issue of hidden momentum, and its counterintuitive dynamical implications, is also analyzed. Finally, a number of issues regarding the electromagnetic interaction and the physical meaning of Dixon's equations are clarified.
Budarin, Vitaliy L; Clark, James H; Deswarte, Fabien E I; Mueller, Karl T; Tavener, Stewart J
2007-06-14
Magic Angle Spinning (MAS) (19)F NMR spectra have been obtained and chemical shifts measured for 37 molecules in the gas phase and adsorbed on the surfaces of six common materials: octadecyl- and octyl-functionalised chromatography silicas, Kieselgel 100 silica, Brockmann neutral alumina, Norit activated charcoal and 3-(1-piperidino)propyl functionalised silica. From these six surfaces, octadecyl-silica is selected as a non-polar reference to which the others are compared. The change in chemical shift of a fluorine nucleus within a molecule on adsorption to a surface from the gas phase, Deltadelta(gas)(surface), is described by the empirical relationship: Deltadelta(gas)(surface) = delta(s) + (alpha(s)+pi(s))/alpha(r) (Deltadelta(gas)(reference) - delta(r)) + delta(HBA) + delta(HBD), where delta(s) and delta(r) are constants that describe the chemical shift induced by the electromagnetic field of the surface under investigation and reference surface, alpha(s) and alpha(r) are the relative surface polarisability for the surface and reference, pi(s) is an additional contribution to the surface polarisabilities due to its ability to interact with aromatic molecules, and delta(HBA) and delta(HBD) are measurements of the hydrogen acceptor and donor properties of the surface. These empirical parameters are measured for the surfaces under study. Silica and alumina are found to undergo specific interactions with aromatic reporter molecules and both accept and donate H-bonds. Activated charcoal was found to have an extreme effect on shielding but no specific interactions with the adsorbed molecules. 3-(1-Piperidino)propyl functionalised silica exhibits H-bond acceptor ability, but does not donate H-bonds. PMID:17487325
Quantum spin dynamics in a spin-orbit-coupled Bose-Einstein condensate
NASA Astrophysics Data System (ADS)
Poon, Ting Fung Jeffrey; Liu, Xiong-Jun
2016-06-01
Spin-orbit-coupled bosons can exhibit rich equilibrium phases at low temperature and in the presence of particle-particle interactions. In the case with a 1D synthetic spin-orbit interaction, it has been observed that the ground state of a Bose gas can be a normal phase, stripe phase, or magnetized phase in different parameter regimes. The magnetized states are doubly degenerate and consist of a many-particle two-state system. In this work, we investigate the nonequilibrium quantum dynamics by switching on a simple one-dimensional optical lattice potential as external perturbation to induce resonant couplings between the magnetized phases, and predict a quantum spin dynamics which cannot be obtained in the single-particle systems. In particular, due to particle-particle interactions, the transition of the Bose condensate from one magnetized phase to the other is forbidden when the external perturbation strength is less than a critical value, and a full transition can occur only when the perturbation exceeds such critical strength. This phenomenon manifests itself a dynamical phase transition, with the order parameter defined by the time-averaged magnetization over an oscillation period, and the critical point behavior being exactly solvable. The thermal fluctuations are also considered in detail. From numerical simulations and exact analytic studies we show that the predicted many-body effects can be well observed with the current experiments.
Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig
NASA Technical Reports Server (NTRS)
Morrison, Carlos R.; Provenza, Andrew; Kurkov, Anatole; Mehmed, Oral; Johnson, Dexter; Montague, Gerald; Duffy, Kirsten; Jansen, Ralph
2005-01-01
The Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig is an apparatus for vibration testing of turbomachine blades in a vacuum at rotational speeds from 0 to 40,000 rpm. This rig includes (1) a vertically oriented shaft on which is mounted an assembly comprising a rotor holding the blades to be tested, (2) two actively controlled heteropolar radial magnetic bearings at opposite ends of the shaft, and (3) an actively controlled magnetic thrust bearing at the upper end of the shaft. This rig is a more capable successor to a prior apparatus, denoted the Dynamic Spin Rig (DSR), that included a vertically oriented shaft with a mechanical thrust bearing at the upper end and a single actively controlled heteropolar radial magnetic bearing at the lower end.
Current-driven spin dynamics in spin-orbit coupled superconductors
NASA Astrophysics Data System (ADS)
Vignale, Giovanni
2012-02-01
The study of the interplay between spin-orbit coupling (SOC) and superconductivity in two-dimensional electron gases (2DEG) has recently gained impetus following the discovery of i) 2DEGs in InAs or GaAs semiconductor heterostructures that are proximized by ordinary s-wave superconducting leads -- a class of systems which plays a key role in the quest for Majorana fermions -- and ii) 2DEGs that form at interfaces between complex oxides such as LaAlO3 and SrTiO3, which display tunable SOC and, under appropriate conditions, superconductivity. Motivated by this body of experimental and theoretical literature, we investigate the collective spin dynamics of an archetypical 2DEG model Hamiltonian with Rashba SOC in the presence of repulsive electron-electron (e-e) interactions. In the absence of superconductivity a Rashba 2DEG exhibits spin oscillations, which, at long wavelength and for weak repulsive interactions, have a frequency 2 αkF, α being the strength of SOC and kF the usual 2D Fermi wavenumber in the absence of SOC. These oscillations, however, are damped and quickly decay due to the emission of (double) electron-hole pairs, which, in the normal phase, are present at arbitrary low energies. In the presence of superconductivity, collective spin oscillations continue to exist in a wide range of parameters, because the Cooper pairs are mixtures of singlet and triplet components. Further, these excitations are undamped because they lie inside the superconducting gap where no other excitation exists. These spin oscillations can be excited by the application of a magnetic field or a supercurrent and can be used to realize persistent spin oscillators operating in the frequency range of 10 GHz - 1 THz.[4pt] Work supported by EU FP7 Programme Grant No. 215368-SEMISPINNET, No. 234970- NANOCTM and No. 248629-SOLID, and by NSF DMR-0705460.
Dynamics of entanglement of two electron spins interacting with nuclear spin baths in quantum dots
NASA Astrophysics Data System (ADS)
Bragar, Igor; Cywiński, Łukasz
2015-04-01
We study the dynamics of entanglement of two electron spins in two quantum dots, in which each electron is interacting with its nuclear spin environment. Focusing on the case of uncoupled dots, and starting from either Bell or Werner states of two qubits, we calculate the decay of entanglement due to the hyperfine interaction with the nuclei. We mostly focus on the regime of magnetic fields in which the bath-induced electron spin flips play a role, for example, their presence leads to the appearance of entanglement sudden death at finite time for two qubits initialized in a Bell state. For these fields, the intrabath dipolar interactions and spatial inhomogeneity of hyperfine couplings are irrelevant on the time scale of coherence (and entanglement) decay, and most of the presented calculations are performed using the uniform-coupling approximation to the exact hyperfine Hamiltonian. We provide a comprehensive overview of entanglement decay in this regime, considering both free evolution of the qubits, and an echo protocol with simultaneous application of π pulses to the two spins. All the currently relevant for experiments bath states are considered: the thermal state, narrowed states (characterized by diminished uncertainty of one of the components of the Overhauser field) of two uncorrelated baths, and a correlated narrowed state with a well-defined value of the z component of the Overhauser field interdot gradient. While we mostly use concurrence to quantify the amount of entanglement in a mixed state of the two electron spins, we also show that their entanglement dynamics can be reconstructed from measurements of the currently relevant for experiments entanglement witnesses and the fidelity of quantum teleportation, performed using a partially disentangled state as a resource.
Demissie, Taye B; Jaszuński, Michał; Komorovsky, Stanislav; Repisky, Michal; Ruud, Kenneth
2015-10-28
We present nuclear spin-rotation constants, absolute nuclear magnetic resonance (NMR) shielding constants, and shielding spans of all the nuclei in (175)LuX and (197)AuX (X = (19)F, (35)Cl, (79)Br, (127)I), calculated using coupled-cluster singles-and-doubles with a perturbative triples (CCSD(T)) correction theory, four-component relativistic density functional theory (relativistic DFT), and non-relativistic DFT. The total nuclear spin-rotation constants determined by adding the relativistic corrections obtained from DFT calculations to the CCSD(T) values are in general in agreement with available experimental data, indicating that the computational approach followed in this study allows us to predict reliable results for the unknown spin-rotation constants in these molecules. The total NMR absolute shielding constants are determined for all the nuclei following the same approach as that applied for the nuclear spin-rotation constants. In most of the molecules, relativistic effects significantly change the computed shielding constants, demonstrating that straightforward application of the non-relativistic formula relating the electronic contribution to the nuclear spin-rotation constants and the paramagnetic contribution to the shielding constants does not yield correct results. We also analyze the origin of the unusually large absolute shielding constant and its relativistic correction of gold in AuF compared to the other gold monohalides. PMID:26520517
NASA Astrophysics Data System (ADS)
Demissie, Taye B.; Jaszuński, Michał; Komorovsky, Stanislav; Repisky, Michal; Ruud, Kenneth
2015-10-01
We present nuclear spin-rotation constants, absolute nuclear magnetic resonance (NMR) shielding constants, and shielding spans of all the nuclei in 175LuX and 197AuX (X = 19F, 35Cl, 79Br, 127I), calculated using coupled-cluster singles-and-doubles with a perturbative triples (CCSD(T)) correction theory, four-component relativistic density functional theory (relativistic DFT), and non-relativistic DFT. The total nuclear spin-rotation constants determined by adding the relativistic corrections obtained from DFT calculations to the CCSD(T) values are in general in agreement with available experimental data, indicating that the computational approach followed in this study allows us to predict reliable results for the unknown spin-rotation constants in these molecules. The total NMR absolute shielding constants are determined for all the nuclei following the same approach as that applied for the nuclear spin-rotation constants. In most of the molecules, relativistic effects significantly change the computed shielding constants, demonstrating that straightforward application of the non-relativistic formula relating the electronic contribution to the nuclear spin-rotation constants and the paramagnetic contribution to the shielding constants does not yield correct results. We also analyze the origin of the unusually large absolute shielding constant and its relativistic correction of gold in AuF compared to the other gold monohalides.
Dynamics of hot random quantum spin chains: from anyons to Heisenberg spins
NASA Astrophysics Data System (ADS)
Parameswaran, Siddharth; Potter, Andrew; Vasseur, Romain
2015-03-01
We argue that the dynamics of the random-bond Heisenberg spin chain are ergodic at infinite temperature, in contrast to the many-body localized behavior seen in its random-field counterpart. First, we show that excited-state real-space renormalization group (RSRG-X) techniques suffer from a fatal breakdown of perturbation theory due to the proliferation of large effective spins that grow without bound. We repair this problem by deforming the SU (2) symmetry of the Heisenberg chain to its `anyonic' version, SU(2)k , where the growth of effective spins is truncated at spin S = k / 2 . This enables us to construct a self-consistent RSRG-X scheme that is particularly simple at infinite temperature. Solving the flow equations, we compute the excited-state entanglement and show that it crosses over from volume-law to logarithmic scaling at a length scale ξk ~eαk3 . This reveals that (a) anyon chains have random-singlet-like excited states for any finite k; and (b) ergodicity is restored in the Heisenberg limit k --> ∞ . We acknowledge support from the Quantum Materials program of LBNL (RV), the Gordon and Betty Moore Foundation (ACP), and UC Irvine startup funds (SAP).
Jankowska, Marzena; Kupka, Teobald; Stobiński, Leszek; Faber, Rasmus; Lacerda, Evanildo G; Sauer, Stephan P A
2016-02-01
Hartree-Fock and density functional theory with the hybrid B3LYP and general gradient KT2 exchange-correlation functionals were used for nonrelativistic and relativistic nuclear magnetic shielding calculations of helium, neon, argon, krypton, and xenon dimers and free atoms. Relativistic corrections were calculated with the scalar and spin-orbit zeroth-order regular approximation Hamiltonian in combination with the large Slater-type basis set QZ4P as well as with the four-component Dirac-Coulomb Hamiltonian using Dyall's acv4z basis sets. The relativistic corrections to the nuclear magnetic shieldings and chemical shifts are combined with nonrelativistic coupled cluster singles and doubles with noniterative triple excitations [CCSD(T)] calculations using the very large polarization-consistent basis sets aug-pcSseg-4 for He, Ne and Ar, aug-pcSseg-3 for Kr, and the AQZP basis set for Xe. For the dimers also, zero-point vibrational (ZPV) corrections are obtained at the CCSD(T) level with the same basis sets were added. Best estimates of the dimer chemical shifts are generated from these nuclear magnetic shieldings and the relative importance of electron correlation, ZPV, and relativistic corrections for the shieldings and chemical shifts is analyzed. PMID:26503739
Controlling the Excited-State Dynamics of Nuclear Spin Isomers Using the Dynamic Stark Effect.
Waldl, Maria; Oppel, Markus; González, Leticia
2016-07-14
Stark control of chemical reactions uses intense laser pulses to distort the potential energy surfaces of a molecule, thus opening new chemical pathways. We use the concept of Stark shifts to convert a local minimum into a local maximum of the potential energy surface, triggering constructive and destructive wave-packet interferences, which then induce different dynamics on nuclear spin isomers in the electronically excited state of a quinodimethane derivative. Model quantum-dynamical simulations on reduced dimensionality using optimized ultrashort laser pulses demonstrate a difference of the excited-state dynamics of two sets of nuclear spin isomers, which ultimately can be used to discriminate between these isomers. PMID:26840424
Dynamics of spin I=3/2 under spin-locking conditions in an ordered environment.
van der Maarel, J R; Jesse, W; Hancu, I; Woessner, D E
2001-08-01
We have derived approximate analytic solutions to the master equation describing the evolution of the spin I=3/2 density operator in the presence of a radio-frequency (RF) field and both static and fluctuating quadrupolar interactions. Spectra resulting from Fourier transformation of the evolutions of the on-resonance spin-locked magnetization into the various coherences display two satellite pairs and, in some cases, a central line. The central line is generally trimodal, consisting of a narrow component related to a slowly relaxing mode and two broad components pertaining to two faster relaxing modes. The rates of the fast modes are sensitive to slow molecular motion. Neither the amplitude nor the width of the narrow component is affected by the magnitude of the static coupling, whereas the corresponding features of the broad components depend in a rather complicated manner on the spin-lock field strength and static quadrupolar interaction. Under certain experimental conditions, the dependencies of the amplitudes on the dynamics are seen to vanish and the relaxation rates reduce to relatively simple expressions. One of the promising emerging features is the fact that the evolutions into the selectively detected quadrupolar spin polarization order and the rank-two double-quantum coherence do not exhibit a slowly relaxing mode and are particularly sensitive to slow molecular motion. Furthermore, these coherences can only be excited in the presence of a static coupling and this makes it possible to discern nuclei in anisotropic from those in isotropic environment. The feasibility of the spin-lock pulse sequences with limited RF power and a nonvanishing average electric field gradient has been demonstrated through experiments on sodium in a dense lyotropic DNA liquid crystal. PMID:11531352
NASA Astrophysics Data System (ADS)
Heisterkamp, F.; Kirstein, E.; Greilich, A.; Zhukov, E. A.; Kazimierczuk, T.; Yakovlev, D. R.; Pawlis, A.; Bayer, M.
2016-02-01
We study the dynamics of optically induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently precessing electron spins in a magnetic field applied in the Voigt geometry. It is detected by nuclei-induced changes in the electron spin coherence signal. This all-optical technique allows us to measure the longitudinal spin relaxation time T1 of the 77Se isotope in a magnetic field range from 10 to 130 mT under illumination. We combine the optical technique with radio frequency methods to address the coherent spin dynamics of the nuclei and measure Rabi oscillations, Ramsey fringes, and the nuclear spin echo. The inhomogeneous spin dephasing time T2* and the spin coherence time T2 of the 77Se isotope are measured. While the T1 time is on the order of several milliseconds, the T2 time is several hundred microseconds. The experimentally determined condition T1≫T2 verifies the validity of the classical model of nuclear spin cooling for describing the optically induced nuclear spin polarization.
Dynamics of Rb and 21Ne spin ensembles interacting by spin exchange with a high Rb magnetic field
NASA Astrophysics Data System (ADS)
Fang, Jiancheng; Chen, Yao; Lu, Yan; Quan, Wei; Zou, Sheng
2016-07-01
We report on the dynamics of spin-polarized Rb and 21Ne ensembles in which the 21Ne spin ensemble in a glass vapor cell experiences a high magnetic field produced by a Rb electron-spin ensemble. The coupled spin ensembles are modeled and the response of the transverse-step magnetic field excitation is solved and studied experimentally. Moreover, we analyze the frequency response of the ensembles to a transverse-oscillating magnetic field. We demonstrate the strong transverse damping and large frequency shift of the 21Ne spin ensemble as the precession frequencies of 21Ne spin and Rb spin match and the magnetic resonance spectroscopies of the two ensembles merge into one. We also demonstrate the operation of the spin ensembles as a self-compensating co-magnetometer that is insensitive to low-frequency magnetic fields that would be useful for rotation rate sensing. For such sensing applications, a large Rb density is achieved to polarize the 21Ne spins. This density leads to a high Rb electron spin magnetic field and we demonstrate its effect on the dynamics of the co-magnetometer.
precession: Dynamics of spinning black-hole binaries with python
NASA Astrophysics Data System (ADS)
Gerosa, Davide; Kesden, Michael
2016-06-01
We present the numerical code precession, a new open-source python module to study the dynamics of precessing black-hole binaries in the post-Newtonian regime. The code provides a comprehensive toolbox to (i) study the evolution of the black-hole spins along their precession cycles, (ii) perform gravitational-wave-driven binary inspirals using both orbit-averaged and precession-averaged integrations, and (iii) predict the properties of the merger remnant through fitting formulas obtained from numerical-relativity simulations. precession is a ready-to-use tool to add the black-hole spin dynamics to larger-scale numerical studies such as gravitational-wave parameter estimation codes, population synthesis models to predict gravitational-wave event rates, galaxy merger trees and cosmological simulations of structure formation. precession provides fast and reliable integration methods to propagate statistical samples of black-hole binaries from/to large separations where they form to/from small separations where they become detectable, thus linking gravitational-wave observations of spinning black-hole binaries to their astrophysical formation history. The code is also a useful tool to compute initial parameters for numerical-relativity simulations targeting specific precessing systems. precession can be installed from the python Package Index, and it is freely distributed under version control on github, where further documentation is provided.
Planar spin-transfer device with dynamical polarizer and analizer
NASA Astrophysics Data System (ADS)
Bazaliy, Yaroslaw; Kravchenko, Anton
2011-03-01
The behavior of the planar spin-transfer devices with monodomain magnetic layers can be described by the macrospin Landau-Lifshitz-Gilbert (LLG) equation with spin-transfer terms. The LLG description of a device with two layers is simplified after applying the overdamped, large easy-plane anisotropy approximation. A decrease of the magnetic layer thickness asymmetry creates a transition from the conventional polarizer-analizer (``fixed layer -- free layer'') operation regime to the regime of the nearly identical magnets. Here electric current leads to a ``Slonczewski windmill'' dynamic state, rather than producing the magnetic switching. The ``windmill'' precession state of a device with two free layers was investigated by numerical solution of the LLG equation.
Dynamic response of an artificial square spin ice
NASA Astrophysics Data System (ADS)
Jungfleisch, M. B.; Zhang, W.; Iacocca, E.; Sklenar, J.; Ding, J.; Jiang, W.; Zhang, S.; Pearson, J. E.; Novosad, V.; Ketterson, J. B.; Heinonen, O.; Hoffmann, A.
2016-03-01
Magnetization dynamics in an artificial square spin-ice lattice made of Ni80Fe20 with magnetic field applied in the lattice plane is investigated by broadband ferromagnetic resonance spectroscopy. The experimentally observed dispersion shows a rich spectrum of modes corresponding to different magnetization states. These magnetization states are determined by exchange and dipolar interaction between individual islands, as is confirmed by a semianalytical model. In the low field regime below 400 Oe a hysteretic behavior in the mode spectrum is found. Micromagnetic simulations reveal that the origin of the observed spectra is due to the initialization of different magnetization states of individual nanomagnets. Our results indicate that it might be possible to determine the spin-ice state by resonance experiments and are a first step towards the understanding of artificial geometrically frustrated magnetic systems in the high-frequency regime.
Phase ordering dynamics in spin-1 ferromagnetic condensates
NASA Astrophysics Data System (ADS)
Williamson, Lewis; Blakie, Peter
2016-05-01
Spinor Bose-Einstein condensates present rich phase diagrams for exploring phase transitions between states with different symmetry properties. In this work we simulate the approach to equilibrium of a spin-1 condensate quenched from an unmagnetised phase to three different ferromagnetic phases. The three ferromagnetic phases have Z2, SO(2) and SO(3) symmetries respectively and possess different conservation laws. Following the quench, domains of magnetization form, with each domain making an independent choice of the symmetry breaking order parameter. These domains grow and compete for the global equilibrium state. We find that this growth follows universal scaling laws and identify the dynamic universality class for each of the three quenches. Polar-core spin-vortices play a crucial role in the phase ordering of the SO(2) system and we identify fractal structures in the domain patterns of the SO(2) and SO(3) systems. We acknowledge support from the Marsden Fund of New Zealand.
NASA Astrophysics Data System (ADS)
Forster, F.; Mühlbacher, M.; Schuh, D.; Wegscheider, W.; Giedke, G.; Ludwig, S.
2015-12-01
The control of nuclear spins in quantum dots is essential to explore their many-body dynamics and exploit their prospects for quantum information processing. We present a unique combination of dynamic nuclear spin polarization and electric-dipole-induced spin resonance in an electrostatically defined double quantum dot (DQD) exposed to the strongly inhomogeneous field of two on-chip nanomagnets. Our experiments provide direct and unrivaled access to the nuclear spin polarization distribution and allow us to establish and characterize multiple fixed points. Further, we demonstrate polarization of the DQD environment by nuclear spin diffusion which significantly stabilizes the nuclear spins inside the DQD.
Dynamic switching of the spin circulation in tapered magnetic nanodisks
NASA Astrophysics Data System (ADS)
Uhlíř, V.; Urbánek, M.; Hladík, L.; Spousta, J.; Im, M.-Y.; Fischer, P.; Eibagi, N.; Kan, J. J.; Fullerton, E. E.; Šikola, T.
2013-05-01
Magnetic vortices are characterized by the sense of in-plane magnetization circulation and by the polarity of the vortex core. With each having two possible states, there are four possible stable magnetization configurations that can be utilized for a multibit memory cell. Dynamic control of vortex core polarity has been demonstrated using both alternating and pulsed magnetic fields and currents. Here, we show controlled dynamic switching of spin circulation in vortices using nanosecond field pulses by imaging the process with full-field soft X-ray transmission microscopy. The dynamic reversal process is controlled by far-from-equilibrium gyrotropic precession of the vortex core, and the reversal is achieved at significantly reduced field amplitudes when compared with static switching. We further show that both the field pulse amplitude and duration required for efficient circulation reversal can be controlled by appropriate selection of the disk geometry.
NASA Astrophysics Data System (ADS)
Melnikov, N. B.; Reser, B. I.; Paradezhenko, G. V.
2016-08-01
To study the spin-density correlations in the ferromagnetic metals above the Curie temperature, we relate the spin correlator and neutron scattering cross-section. In the dynamic spin-fluctuation theory, we obtain explicit expressions for the effective and local magnetic moments and spatial spin-density correlator. Our theoretical results are demonstrated by the example of bcc Fe. The effective and local moments are found in good agreement with results of polarized neutron scattering experiment over a wide temperature range. The calculated short-range order is small (up to 4 Å) and slowly decreases with temperature.
The effect of iron spin transition on convective dynamics, slab dynamics and the geoid
NASA Astrophysics Data System (ADS)
Jacobs, Michael; van den Berg, Arie; Spakman, Wim; Cadek, Ondrej; Cizkova, Hana; Matyska, Ctirad
2013-04-01
Iron bearing minerals in the Earths lower mantle show a transition from high-spin to low-spin in the iron constituent. This has been observed in particular for ferropericlase both experimentally (Fei et al, 2007, Lin et al. 2005) and in first principles calculations (Wu et al, 2009). The situation is less unambiguous for perovskite. Umemoto et al (2010) showed that the effect on volume is small compared to experimental uncertainty. Therefore we only considered the spin effects in ferropericlase in our models. The spin transition is characterized by a high valued positive Clapeyron slope ? = 19MPa-K while the smoothness of the transition increases with temperature. Fei et al. (2007) showed that at room temperature the spin transition pressure for iron richer composition occurs at higher values, e.g 40 GPa at 20 mol% FeO, 60 GPa at 40 mol% FeO. In order to get a full thermodynamic description of mantle material that includes the effects of spin transitions in ferropericlase we developed a model based on the multi-Einstein vibrational model approach of Jacobs et al. (2013). This model represents volume-pressure data of Lin et al. (2005), spin fraction data predicted by Wu et al. (2009) and it also includes the observed composition dependence of the spin transition pressure. Our new model further includes the thermodynamic description of Jacobs and de Jong (2007) that has been extended to describe thermodynamic properties of iron bearing (Mg,Fe)SiO3 perovskite. Because the spin transition pressure is composition dependent, the spin transition results in the formation of miscibility gap regions separating compositions enriched in high spin and compositions enriched in low-spin state. The spin transition affects thermodynamic properties, density, thermal expansivity, bulk modulus and heat capacity which in turn impact the convection dynamics of the Earth mantle. For instance, due to the high positive Clapeyron-slope of the transition convective mixing becomes more
On the Spin-axis Dynamics of the Earth
NASA Astrophysics Data System (ADS)
Li, Gongjie; Batygin, Konstantin
2015-05-01
The variation of a planet's obliquity is influenced by the existence of satellites with a high mass ratio. For instance, the Earth's obliquity is stabilized by the Moon, and would undergo chaotic variations in the Moon's absence. In turn, such variations can lead to large-scale changes in the atmospheric circulation, rendering spin-axis dynamics a central issue for understanding climate. The relevant quantity for dynamically-forced climate change is the rate of chaotic diffusion. Accordingly, here we reexamine the spin-axis evolution of a Moonless Earth within the context of a simplified perturbative framework. We present analytical estimates of the characteristic Lyapunov coefficient as well as the chaotic diffusion rate and demonstrate that even in absence of the Moon, the stochastic change in the Earth's obliquity is sufficiently slow to not preclude long-term habitability. Our calculations are consistent with published numerical experiments and illustrate the putative system's underlying dynamical structure in a simple and intuitive manner. In addition, we examine if at any point in the Earth's evolutionary history, the obliquity varied significantly. We find that even though the orbital perturbations were different in the past, the system nevertheless avoided resonant encounters throughout its evolution. This indicates that the Earth obtained its current obliquity during the formation of the Moon.
Spin-state configuration induced faster spin dynamics in epitaxial La1-xSrxCoO3 thin films
NASA Astrophysics Data System (ADS)
Cui, W. Y.; Li, P.; Bai, H. L.
2015-05-01
Two important features: spin-state configuration and spin dynamics in phase-separated ferromagnetic/spin-glass epitaxial La1-xSrxCoO3 thin films (x=0.07, 0.17, 0.26, 0.30, 0.40, 0.60) have been investigated and elaborated, proved by both magnetic analyses and first principle calculations. The configuration with high-spin (HS) state Co3+ and low-spin (LS) state Co4+ is considered to be the most stable spin-state configuration for La1-xSrxCoO3 at ground state, which was demonstrated by calculating the magnetic moments of La1-xSrxCoO3, as well as first principle calculation. The stretched Co-O bond by Sr doping causes the decrease of crystal field splitting, resulting in the HS state Co3+ and LS state Co4+. The spin dynamics in the La1-xSrxCoO3 thin films was found to be faster than the classic spin-glass compounds, which is attributed to the higher-spin Co3+, and rather smaller ferromagnetic cluster size (~2.16 to ~21.5 nm) in the epitaxial films than that in referenced polycrystalline compounds (~35 to ~240 nm).
Dynamics of a resonantly driven two-spin system
Volkov, Yu. S. Sinitsyn, D. O.
2007-12-15
Dynamics of a coupled two-spin system in a static magnetic field are investigated. An analysis is presented of resonance transitions driven by a circularly polarized radio-frequency (RF) field orthogonal to the static field. When the RF field amplitude is modulated at a certain frequency depending on the field strength, the system exhibits parametric resonance behavior. The periodicity of transitions breaks down, and the Shannon entropy of the recurrence probability density for the system's states increases by more than an order of magnitude.
Experimental investigation of the dynamics of spinning tethered bodies
NASA Astrophysics Data System (ADS)
Modi, V. J.; Pradhan, S.; Chu, M.; Tyc, G.; Misra, A. K.
1996-10-01
Ground based experiments are conducted as a part of the OEDIPUS-C sounding rocket mission, scheduled for launch in the winter of 1995. Here OEDIPUS stands for Observation of Electrified Distribution in Ionospheric Plasma—a Unique Strategy. The OEDIPUS-C configuration consists of two spinning bodies connected by a 1 km long tether (the spin axis is nominally along the tether line). The objective is to assess dynamic behaviour of the tether and the payload. The test configuration consists of an end-body supported by a tether. The test procedure involves slow spin-up of the system and identifying the speeds corresponding to onset of the tether modes or the large amplitude end-body coning. This is referred to as the critical speed and corresponds to the stability boundary of the system. Experimental results are obtained for four different bodies to study the system stability over a wide range of mass and geometric parameters. Effect of offset of the tether attachment from the end-body centre of mass is also investigated. The observed critical speeds are compared with those given by the linear theory. The test results are generally in very good agreement with the theory, however several transient phenomena observed during the test suggest that system nonlinearities cannot be ignored when modelling such a complex system.
Spin-down Dynamics of Magnetized Solar-type Stars
NASA Astrophysics Data System (ADS)
Oglethorpe, R. L. F.; Garaud, P.
2013-12-01
It has long been known that solar-type stars undergo significant spin-down, via magnetic braking, during their main-sequence lifetimes. However, magnetic braking only operates on the surface layers; it is not yet completely understood how angular momentum is transported within the star and how rapidly the spin-down information is communicated to the deep interior. In this work, we use insight from recent progress in understanding internal solar dynamics to model the interior of other solar-type stars. We assume, following Gough & McIntyre, that the bulk of the radiation zone of these stars is held in uniform rotation by the presence of an embedded large-scale primordial field, confined below a stably stratified, magnetic-free tachocline by large-scale meridional flows downwelling from the convection zone. We derive simple equations to describe the response of this model interior to spin-down of the surface layers, which are identical to the two-zone model of MacGregor & Brenner, with a coupling timescale proportional to the local Eddington-Sweet timescale across the tachocline. This timescale depends both on the rotation rate of the star and on the thickness of the tachocline, and it can vary from a few hundred thousand years to a few Gyr, depending on stellar properties. Qualitative predictions of the model appear to be consistent with observations, although they depend sensitively on the assumed functional dependence of the tachocline thickness on the stellar rotation rate.
Experimental test of the Chao matrix formalism for spin dynamics.
NASA Astrophysics Data System (ADS)
Morozov, V. S.; Chao, A. W.; Krisch, A. D.; Leonova, M. A.; Raymond, R. S.; Sivers, D. W.; Wong, V. K.; Gebel, R.; Lehrach, A.; Lorentz, B.; Maier, R.; Prasuhn, D.; Schnase, A.; Stockhorst, H.; Hinterberger, F.; Ulbrich, K.
2007-04-01
We recently started testing Chao's proposed new matrix formalism for describing the spin dynamics due to a single spin resonance in a stored polarized beam. This formalism seems to be the first generalization of the Froissart-Stora equation since it was published in 1960. It allows one to calculate analytically the polarization's behavior inside a resonance, which is not possible using the Froissart-Stora equation. We recently tested some Chao formalism predictions using a 1.85 GeV/c polarized deuteron beam stored in COSY. We swept an rf dipole's frequency through 200 Hz, at different sweep rates, while varying the distance from the sweep's end frequency to an rf-induced spin resonance's central frequency. We compared our experimental data with the predictions of the Chao formalism and the prediction of a phenomenological Froissart-Stora-based two-fluid model. The Froissart-Stora formula itself can make no prediction inside the resonance. The data seem to support the validity of the Chao formalism. (Supported by the German BMBF Science Ministry.)
Skyrmion dynamics in chiral ferromagnets under spin-transfer torque
NASA Astrophysics Data System (ADS)
Komineas, Stavros; Papanicolaou, Nikos
2015-11-01
We study the dynamics of skyrmions under spin-transfer torque in Dzyaloshinskii-Moriya materials with easy-axis anisotropy. In particular, we study the motion of a topological skyrmion with skyrmion number Q =1 and a nontopological skyrmionium with Q =0 using their linear momentum, virial relations, and numerical simulations. The nontopological Q =0 skyrmionium is accelerated in the direction of the current flow and it either reaches a steady state with constant velocity, or it is elongated to infinity. The steady-state velocity is given by a balance between current and dissipation and has an upper limit. In contrast, the topological Q =1 skyrmion converges to a steady state with constant velocity at an angle to the current flow. When the spin current stops the Q =1 skyrmion is spontaneously pinned, whereas the Q =0 skyrmionium continues propagation. Exact solutions for the propagating skyrmionium are identified as solutions of equations given numerically in a previous work. Further exact results for propagating skyrmions are given in the case of the pure exchange model. The traveling solutions provide arguments that a spin-polarized current will cause rigid motion of a skyrmion or a skyrmionium.
Dynamics of the two-spin spin-boson model with a common bath.
Deng, Tianrui; Yan, Yiying; Chen, Lipeng; Zhao, Yang
2016-04-14
Dynamics of the two-spin spin-boson model in the presence of Ohmic and sub-Ohmic baths is investigated by employing a multitude of the Davydov D1 trial states, also known as the multi-D1 Ansatz. Its accuracy in dynamics simulations of the two-spin SBM is improved significantly over the single D1 Ansatz, especially in the weak to moderately strong coupling regime. Validity of the multi-D1 Ansatz for various coupling strengths is also systematically examined by making use of the deviation vector which quantifies how faithfully the trial state obeys the Schrödinger equation. The time evolution of population difference and entanglement has been studied for various initial conditions and coupling strengths. Careful comparisons are carried out between our approach and three other methods, i.e., the time-dependent numerical renormalization group (TD-NRG) approach, the Bloch-Redfield theory, and a method based on a variational master equation. For strong coupling, the multi-D1 trial state yields consistent results as the TD-NRG approach in the Ohmic regime while the two disagree in the sub-Ohmic regime, where the multi-D1 trial state is shown to be more accurate. For weak coupling, the multi-D1 trial state agrees with the two master-equation methods in the presence of both Ohmic and sub-Ohmic baths, but shows considerable differences with the TD-NRG approach in the presence of a sub-Ohmic bath, calling into question the validity of the TD-NRG results at long times in the literature. PMID:27083703
Dynamics of the two-spin spin-boson model with a common bath
NASA Astrophysics Data System (ADS)
Deng, Tianrui; Yan, Yiying; Chen, Lipeng; Zhao, Yang
2016-04-01
Dynamics of the two-spin spin-boson model in the presence of Ohmic and sub-Ohmic baths is investigated by employing a multitude of the Davydov D1 trial states, also known as the multi-D1 Ansatz. Its accuracy in dynamics simulations of the two-spin SBM is improved significantly over the single D1 Ansatz, especially in the weak to moderately strong coupling regime. Validity of the multi-D1 Ansatz for various coupling strengths is also systematically examined by making use of the deviation vector which quantifies how faithfully the trial state obeys the Schrödinger equation. The time evolution of population difference and entanglement has been studied for various initial conditions and coupling strengths. Careful comparisons are carried out between our approach and three other methods, i.e., the time-dependent numerical renormalization group (TD-NRG) approach, the Bloch-Redfield theory, and a method based on a variational master equation. For strong coupling, the multi-D1 trial state yields consistent results as the TD-NRG approach in the Ohmic regime while the two disagree in the sub-Ohmic regime, where the multi-D1 trial state is shown to be more accurate. For weak coupling, the multi-D1 trial state agrees with the two master-equation methods in the presence of both Ohmic and sub-Ohmic baths, but shows considerable differences with the TD-NRG approach in the presence of a sub-Ohmic bath, calling into question the validity of the TD-NRG results at long times in the literature.
Exact spin dynamics of inhomogeneous 1-d systems at high temperature
NASA Astrophysics Data System (ADS)
Danieli, E. P.; Pastawski, H. M.; Levstein, P. R.
2002-07-01
The evaluation of spin excitation dynamics in finite 1-d systems of spins {1}/{2} with XY exchange interaction J acquired new interest because NMR experiments at high temperature ( kBT≫ J) confirmed the predicted spin wave behavior of mesoscopic echoes. In this work, we use the Jordan-Wigner transformation to obtain the exact dynamics of inhomogeneous chains and rings where the evolution is reduced to one-body dynamics. For higher dimensions, the spin excitations manifest many-body effects that can be interpreted as a simple dynamics of non-interacting fermions plus a decoherent process.
Information-flux approach to multiple-spin dynamics
NASA Astrophysics Data System (ADS)
di Franco, C.; Paternostro, M.; Palma, G. M.; Kim, M. S.
2007-10-01
We introduce and formalize the concept of information flux in a many-body register as the influence that the dynamics of a specific element receive from any other element of the register. By quantifying the information flux in a protocol, we can design the most appropriate initial state of the system and, noticeably, the distribution of coupling strengths among the parts of the register itself. The intuitive nature of this tool and its flexibility, which allow for easily manageable numerical approaches when analytic expressions are not straightforward, are greatly useful in interacting many-body systems such as quantum spin chains. We illustrate the use of this concept in quantum cloning and quantum state transfer and we also sketch its extension to nonunitary dynamics.
Information-flux approach to multiple-spin dynamics
Di Franco, C.; Paternostro, M.; Kim, M. S.; Palma, G. M.
2007-10-15
We introduce and formalize the concept of information flux in a many-body register as the influence that the dynamics of a specific element receive from any other element of the register. By quantifying the information flux in a protocol, we can design the most appropriate initial state of the system and, noticeably, the distribution of coupling strengths among the parts of the register itself. The intuitive nature of this tool and its flexibility, which allow for easily manageable numerical approaches when analytic expressions are not straightforward, are greatly useful in interacting many-body systems such as quantum spin chains. We illustrate the use of this concept in quantum cloning and quantum state transfer and we also sketch its extension to nonunitary dynamics.
Spin glass model for dynamics of cell reprogramming
NASA Astrophysics Data System (ADS)
Pusuluri, Sai Teja; Lang, Alex H.; Mehta, Pankaj; Castillo, Horacio E.
2015-03-01
Recent experiments show that differentiated cells can be reprogrammed to become pluripotent stem cells. The possible cell fates can be modeled as attractors in a dynamical system, the ``epigenetic landscape.'' Both cellular differentiation and reprogramming can be described in the landscape picture as motion from one attractor to another attractor. We perform Monte Carlo simulations in a simple model of the landscape. This model is based on spin glass theory and it can be used to construct a simulated epigenetic landscape starting from the experimental genomic data. We re-analyse data from several cell reprogramming experiments and compare with our simulation results. We find that the model can reproduce some of the main features of the dynamics of cell reprogramming.
Dynamical spin structure factor of one-dimensional interacting fermions
NASA Astrophysics Data System (ADS)
Zyuzin, Vladimir A.; Maslov, Dmitrii L.
2015-02-01
We revisit the dynamic spin susceptibility χ (q ,ω ) of one-dimensional interacting fermions. To second order in the interaction, backscattering results in a logarithmic correction to χ (q ,ω ) at q ≪kF , even if the single-particle spectrum is linearized near the Fermi points. Consequently, the dynamic spin structure factor Im χ (q ,ω ) is nonzero at frequencies above the single-particle continuum. In the boson language, this effect results from the marginally irrelevant backscattering operator of the sine-Gordon model. Away from the threshold, the high-frequency tail of Im χ (q ,ω ) due to backscattering is larger than that due to finite mass by a factor of kF/q . We derive the renormalization group equations for the coupling constants of the g -ology model at finite ω and q and find the corresponding expression for χ (q ,ω ) , valid to all orders in the interaction but not in the immediate vicinity of the continuum boundary, where the finite-mass effects become dominant.
Quenching of dynamic nuclear polarization by spin-orbit coupling in GaAs quantum dots.
Nichol, John M; Harvey, Shannon P; Shulman, Michael D; Pal, Arijeet; Umansky, Vladimir; Rashba, Emmanuel I; Halperin, Bertrand I; Yacoby, Amir
2015-01-01
The central-spin problem is a widely studied model of quantum decoherence. Dynamic nuclear polarization occurs in central-spin systems when electronic angular momentum is transferred to nuclear spins and is exploited in quantum information processing for coherent spin manipulation. However, the mechanisms limiting this process remain only partially understood. Here we show that spin-orbit coupling can quench dynamic nuclear polarization in a GaAs quantum dot, because spin conservation is violated in the electron-nuclear system, despite weak spin-orbit coupling in GaAs. Using Landau-Zener sweeps to measure static and dynamic properties of the electron spin-flip probability, we observe that the size of the spin-orbit and hyperfine interactions depends on the magnitude and direction of applied magnetic field. We find that dynamic nuclear polarization is quenched when the spin-orbit contribution exceeds the hyperfine, in agreement with a theoretical model. Our results shed light on the surprisingly strong effect of spin-orbit coupling in central-spin systems. PMID:26184854
Quenching of dynamic nuclear polarization by spin-orbit coupling in GaAs quantum dots
NASA Astrophysics Data System (ADS)
Nichol, John M.; Harvey, Shannon P.; Shulman, Michael D.; Pal, Arijeet; Umansky, Vladimir; Rashba, Emmanuel I.; Halperin, Bertrand I.; Yacoby, Amir
2015-07-01
The central-spin problem is a widely studied model of quantum decoherence. Dynamic nuclear polarization occurs in central-spin systems when electronic angular momentum is transferred to nuclear spins and is exploited in quantum information processing for coherent spin manipulation. However, the mechanisms limiting this process remain only partially understood. Here we show that spin-orbit coupling can quench dynamic nuclear polarization in a GaAs quantum dot, because spin conservation is violated in the electron-nuclear system, despite weak spin-orbit coupling in GaAs. Using Landau-Zener sweeps to measure static and dynamic properties of the electron spin-flip probability, we observe that the size of the spin-orbit and hyperfine interactions depends on the magnitude and direction of applied magnetic field. We find that dynamic nuclear polarization is quenched when the spin-orbit contribution exceeds the hyperfine, in agreement with a theoretical model. Our results shed light on the surprisingly strong effect of spin-orbit coupling in central-spin systems.
Non-diffusive spin dynamics in a two-dimensional electron gas
Weber, C.P.
2010-04-28
We describe measurements of spin dynamics in the two-dimensional electron gas in GaAs/GaAlAs quantum wells. Optical techniques, including transient spin-grating spectroscopy, are used to probe the relaxation rates of spin polarization waves in the wavevector range from zero to 6 x 10{sup 4} cm{sup -1}. We find that the spin polarization lifetime is maximal at nonzero wavevector, in contrast with expectation based on ordinary spin diffusion, but in quantitative agreement with recent theories that treat diffusion in the presence of spin-orbit coupling.
Non-diffusive spin dynamics in a two-dimensional electrongas
Weber, Christopher P.; Orenstein, Joseph; Bernevig, B. Andrei; Zhang, Shou-Cheng; Stephens, Jason; Awschalom, David D.
2006-12-12
We describe measurements of spin dynamics in thetwo-dimensional electron gas in GaAs/GaAlAs quantum wells. Opticaltechniques, including transient spin-grating spectroscopy, are used toprobe the relaxation rates of spin polarization waves in the wavevectorrange from zero to 6E4 cm-1. We find that the spin polarization lifetimeis maximal at nonzero wavevector, in contrast with expectation based onordinary spin diffusion, but in quantitative agreement with recenttheories that treat diffusion in the presence of spin-orbitcoupling.
Baranowski, M.; Misiewicz, J.
2015-10-21
We report theoretical studies of spin polarization dynamics in dilute nitride semiconductors. We develop a commonly used rate equation model [Lagarde et al., Phys. Status Solidi A 204, 208 (2007) and Kunold et al. Phys. Rev. B 83, 165202 (2011)] to take into account the influence of shallow localizing states on the temperature dependence of spin polarization dynamics and a spin filtering effect. Presented investigations show that the experimentally observed temperature dependence of a spin polarization lifetime in dilute nitrides can be related to the electron capture process by shallow localizing states without paramagnetic properties. This process reduces the efficiency of spin filtering effect by deep paramagnetic centers, especially at low temperatures.
Dynamical spin injection at a quasi-one-dimensional ferromagnet-graphene interface
Singh, S.; Ahmadi, A.; Mucciolo, E. R.; Barco, E. del; Cherian, C. T.; Özyilmaz, B.
2015-01-19
We present a study of dynamical spin injection from a three-dimensional ferromagnet into two-dimensional single-layer graphene. Comparative ferromagnetic resonance (FMR) studies of ferromagnet/graphene strips buried underneath the central line of a coplanar waveguide show that the FMR linewidth broadening is the largest when the graphene layer protrudes laterally away from the ferromagnetic strip, indicating that the spin current is injected into the graphene areas away from the area directly underneath the ferromagnet being excited. Our results confirm that the observed damping is indeed a signature of dynamical spin injection, wherein a pure spin current is pumped into the single-layer graphene from the precessing magnetization of the ferromagnet. The observed spin pumping efficiency is difficult to reconcile with the expected backflow of spins according to the standard spin pumping theory and the characteristics of graphene, and constitutes an enigma for spin pumping in two-dimensional structures.
Lattice dynamics in spin-crossover nanoparticles through nuclear inelastic scattering
NASA Astrophysics Data System (ADS)
Félix, Gautier; Mikolasek, Mirko; Peng, Haonan; Nicolazzi, William; Molnár, Gábor; Chumakov, Aleksandr I.; Salmon, Lionel; Bousseksou, Azzedine
2015-01-01
We used nuclear inelastic scattering (NIS) to investigate the lattice dynamics in [Fe(pyrazine)(Ni(CN)4)] spin crossover nanoparticles. The vibrational density of states of iron was extracted from the NIS data, which allowed to determine characteristic thermodynamical and lattice dynamical parameters as well as their spin-state dependence. The optical part of the NIS spectra compares well with the Raman scattering data reflecting the expansion/contraction of the coordination octahedron during the spin transition. From the acoustic part, we extracted the sound velocity in the low-spin (vLS=2073 ±31 m s-1) and high-spin (vHS=1942 ±23 m s-1) states of the particles. The spin-state dependence of this parameter is of primary interest to rationalize the spin-transition behavior in solids as well as its dynamics and finite size effects.
Strain dependent electron spin dynamics in bulk cubic GaN
Schaefer, A.; Buß, J. H.; Hägele, D.; Rudolph, J.; Schupp, T.; Zado, A.; As, D. J.
2015-03-07
The electron spin dynamics under variable uniaxial strain is investigated in bulk cubic GaN by time-resolved magneto-optical Kerr-rotation spectroscopy. Spin relaxation is found to be approximately independent of the applied strain, in complete agreement with estimates for Dyakonov-Perel spin relaxation. Our findings clearly exclude strain-induced relaxation as an effective mechanism for spin relaxation in cubic GaN.
Spin probe dynamics of n-hexadecane in confined geometry
NASA Astrophysics Data System (ADS)
Lukešová, Miroslava; Švajdlenková, Helena; Sippel, Pit; Macová, Eva; Berek, Dušan; Loidl, Alois; Bartoš, Josef
2015-02-01
A combined study of the rotational dynamics of the stable free radical 2,2,6,6-tetramethyl-1-piperidinyloxy (TEMPO) and the phase behavior of n-hexadecane (n-HXD) in the bulk and the confined states in a series of silica gels (SG) by means of ESR and DSC is presented. A slow to fast motion transition of the spin probe TEMPO in the bulk n-HXD occurs at T50 G,bulk ≪ Tm,bulk, i.e., well below the melting temperature due to its trapping and localized mobility in the interlamellar gap of the crystallites [J. Bartoš, H. Švajdlenková, M. Zaleski, M. Edelmann, M. Lukešová, Physica B 430, 99 (2013)]. On the other hand, the dynamics of the TEMPO in the confined systems is strongly slowing down with T50 G (Dpore) >Tm(Dpore) and slightly increases with the pore size Dpore = 60, 100 and 300 Å of the SG's. At the same time, both the corresponding melting temperature, Tm (Dpore), and melting enthalpy, ΔHm (Dpore), decrease with Dpore together with the mutual anti-correlation between T50 G and Tm as a function of the inverse of pore diameter, 1/Dpore. Moreover, the dynamic heterogeneity of the TEMPO in the confined state below T50 G (Dpore) is closely related to the phase transformation. The strong slowing down of the spin probe motion likely results from its preferential localization at the interface layer of the matrix pore due to specific interaction of TEMPO molecules with the polar silanol groups of the SG matrix. This is supported by special study on a series of the variously filled n-HXD/SG systems, other similar experimental findings as well as by theoretical spectral argument.
Spin dynamics in relativistic ionization with highly charged ions in super-strong laser fields
NASA Astrophysics Data System (ADS)
Klaiber, Michael; Yakaboylu, Enderalp; Müller, Carsten; Bauke, Heiko; Paulus, Gerhard G.; Hatsagortsyan, Karen Z.
2014-03-01
Spin dynamics and induced spin effects in above-threshold ionization of hydrogenlike highly charged ions in super-strong laser fields are investigated. Spin-resolved ionization rates in the tunnelling regime are calculated by employing two versions of a relativistic Coulomb-corrected strong-field approximation (SFA). An intuitive simpleman model is developed which explains the derived scaling laws for spin flip and spin asymmetry effects. The intuitive model as well as our ab initio numerical simulations support the analytical results for the spin effects obtained in the dressed SFA where the impact of the laser field on the electron spin evolution in the bound state is taken into account. In contrast, the standard SFA is shown to fail in reproducing spin effects in ionization even at a qualitative level. The anticipated spin-effects are expected to be measurable with modern laser techniques combined with an ion storage facility.
Solid effect in magic angle spinning dynamic nuclear polarization
NASA Astrophysics Data System (ADS)
Corzilius, Björn; Smith, Albert A.; Griffin, Robert G.
2012-08-01
For over five decades, the solid effect (SE) has been heavily utilized as a mechanism for performing dynamic nuclear polarization (DNP). Nevertheless, it has not found widespread application in contemporary, high magnetic field DNP experiments because SE enhancements display an ω _0 ^{ - 2} field dependence. In particular, for nominally forbidden zero and double quantum SE transitions to be partially allowed, it is necessary for mixing of adjacent nuclear spin states to occur, and this leads to the observed field dependence. However, recently we have improved our instrumentation and report here an enhancement of ɛ = 91 obtained with the organic radical trityl (OX063) in magic angle spinning experiments performed at 5 T and 80 K. This is a factor of 6-7 higher than previous values in the literature under similar conditions. Because the solid effect depends strongly on the microwave field strength, we attribute this large enhancement to larger microwave field strengths inside the sample volume, achieved with more efficient coupling of the gyrotron to the sample chamber. In addition, we develop a theoretical model to explain the dependence of the buildup rate of enhanced nuclear polarization and the steady-state enhancement on the microwave power. Buildup times and enhancements were measured as a function of 1H concentration for both trityl and Gd-DOTA. Comparison of the results indicates that for trityl the initial polarization step is the slower, rate-determining step. However, for Gd-DOTA the spread of nuclear polarization via homonuclear 1H spin diffusion is rate-limiting. Finally, we discuss the applicability of the solid effect at fields > 5 T and the requirements to address the unfavorable field dependence of the solid effect.
Solid effect in magic angle spinning dynamic nuclear polarization
Corzilius, Björn; Smith, Albert A.; Griffin, Robert G.
2012-01-01
For over five decades, the solid effect (SE) has been heavily utilized as a mechanism for performing dynamic nuclear polarization (DNP). Nevertheless, it has not found widespread application in contemporary, high magnetic field DNP experiments because SE enhancements display an \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{upgreek} \\usepackage{mathrsfs} \\setlength{\\oddsidemargin}{-69pt} \\begin{document} \\begin{equation*}\\omega _0 ^{ - 2}\\end{equation*} \\end{document}ω0−2 field dependence. In particular, for nominally forbidden zero and double quantum SE transitions to be partially allowed, it is necessary for mixing of adjacent nuclear spin states to occur, and this leads to the observed field dependence. However, recently we have improved our instrumentation and report here an enhancement of ɛ = 91 obtained with the organic radical trityl (OX063) in magic angle spinning experiments performed at 5 T and 80 K. This is a factor of 6-7 higher than previous values in the literature under similar conditions. Because the solid effect depends strongly on the microwave field strength, we attribute this large enhancement to larger microwave field strengths inside the sample volume, achieved with more efficient coupling of the gyrotron to the sample chamber. In addition, we develop a theoretical model to explain the dependence of the buildup rate of enhanced nuclear polarization and the steady-state enhancement on the microwave power. Buildup times and enhancements were measured as a function of 1H concentration for both trityl and Gd-DOTA. Comparison of the results indicates that for trityl the initial polarization step is the slower, rate-determining step. However, for Gd-DOTA the spread of nuclear polarization via homonuclear 1H spin diffusion is rate-limiting. Finally, we discuss the applicability of the solid effect at fields > 5 T and the requirements
Solid effect in magic angle spinning dynamic nuclear polarization.
Corzilius, Björn; Smith, Albert A; Griffin, Robert G
2012-08-01
For over five decades, the solid effect (SE) has been heavily utilized as a mechanism for performing dynamic nuclear polarization (DNP). Nevertheless, it has not found widespread application in contemporary, high magnetic field DNP experiments because SE enhancements display an ω(0)(-2) field dependence. In particular, for nominally forbidden zero and double quantum SE transitions to be partially allowed, it is necessary for mixing of adjacent nuclear spin states to occur, and this leads to the observed field dependence. However, recently we have improved our instrumentation and report here an enhancement of ε = 91 obtained with the organic radical trityl (OX063) in magic angle spinning experiments performed at 5 T and 80 K. This is a factor of 6-7 higher than previous values in the literature under similar conditions. Because the solid effect depends strongly on the microwave field strength, we attribute this large enhancement to larger microwave field strengths inside the sample volume, achieved with more efficient coupling of the gyrotron to the sample chamber. In addition, we develop a theoretical model to explain the dependence of the buildup rate of enhanced nuclear polarization and the steady-state enhancement on the microwave power. Buildup times and enhancements were measured as a function of (1)H concentration for both trityl and Gd-DOTA. Comparison of the results indicates that for trityl the initial polarization step is the slower, rate-determining step. However, for Gd-DOTA the spread of nuclear polarization via homonuclear (1)H spin diffusion is rate-limiting. Finally, we discuss the applicability of the solid effect at fields > 5 T and the requirements to address the unfavorable field dependence of the solid effect. PMID:22894339
R.C. Quittmeyer
2005-11-16
The purpose of the drip shield (DS) is to divert water that may seep into emplacement drifts from contacting the waste packages, and to protect the waste packages from impact or static loading from rockfall. The objective of this document is to summarize, into one location, the results of a series of supporting engineering calculations that were developed to study the effect of static and dynamic loads on the mechanical performance of the DS. The potential DS loads are a result of: (1) Potential earthquake vibratory ground motion, and resulting interaction of the DS, waste package and pallet, and drift invert; (2) Dynamic impacts of rockfall resulting from emplacement drift damage as a result of earthquake vibratory motion; and (3) Static load of the caved rock rubble that may come to rest on the DS as a result of vibratory motion or from time-dependent yielding of the rock mass surrounding the emplacement drift. The potential mechanical failure mechanisms that may result from these loads include: (1) Overturning and/or separation of the interlocking DS segments; (2) Loss of structural integrity and stability of the DS, including excessive deformation or buckling; and (3) Localized damage to the top and side-wall plates of the DS. The scope of this document is limited to summarizing results presented in the supporting calculations in the areas of analysis of the potential for DS collapse, and determination of the damaged surface area of the DS plates. New calculations are presented to determine whether or not separation of DSs occur under vibratory motion.
Real time dynamic behavior of vertex frustrated artificial spin ice
NASA Astrophysics Data System (ADS)
Lao, Yuyang; Sklenar, Joseph; Gilbert, Ian; Carrasquilo, Isaac; Scholl, Andreas; Young, Anthony; Nisoli, Cristiano; Schiffer, Peter
Artificial spin ice systems comprise two dimensional arrays of nanoscale single domain ferromagnets designed to have frustrated interactions among the moments. By decimating islands from the common square artificial spin ice, one can design lattices with so called `vertex frustration'. In such lattices, the geometry prevents all vertices from occupying local ground states simultaneously. Using Photoemission Electron Microscopy (PEEM), we access the real time thermally induced dynamics of the moment behavior in those lattices. Operating at a proper temperature, the moment direction of each island fluctuates with a sufficiently slow frequency that it can be resolvable by acquiring successive PEEM images. We can extract information regarding the collective excitations of the moments and understand how they reflect the frustration of lattice. Supported by the US Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division under Grant No. DE-SC0010778. The work of C.N. was carried out under the auspices of the US Department of Energy at LANL under Contract no. DE-AC52-06NA253962. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract no. DE-AC02-05CH11231.
Manipulating magnetic anisotropy and ultrafast spin dynamics of magnetic nanostructures
NASA Astrophysics Data System (ADS)
Cheng, Zhao-Hua; He, Wei; Zhang, Xiang-Qun; Sun, Da-Li; Du, Hai-Feng; Wu, Qiong; Ye, Jun; Fang, Ya-Peng; Liu, Hao-Liang
2015-07-01
We present our extensive research into magnetic anisotropy. We tuned the terrace width of Si(111) substrate by a novel method: varying the direction of heating current and consequently manipulating the magnetic anisotropy of magnetic structures on the stepped substrate by decorating its atomic steps. Laser-induced ultrafast demagnetization of a CoFeB/MgO/CoFeB magnetic tunneling junction was explored by the time-resolved magneto-optical Kerr effect (TR-MOKE) for both the parallel state (P state) and the antiparallel state (AP state) of the magnetizations between two magnetic layers. It was observed that the demagnetization time is shorter and the magnitude of demagnetization is larger in the AP state than those in the P state. These behaviors are attributed to the ultrafast spin transfer between two CoFeB layers via the tunneling of hot electrons through the MgO barrier. Our observation indicates that ultrafast demagnetization can be engineered by the hot electron tunneling current. This opens the door to manipulate the ultrafast spin current in magnetic tunneling junctions. Furthermore, an all-optical TR-MOKE technique provides the flexibility for exploring the nonlinear magnetization dynamics in ferromagnetic materials, especially with metallic materials. Project supported by the National Basic Research Program of China (Grant Nos. 2015CB921403, 2011CB921801, and 2012CB933101) and the National Natural Science Foundation of China (Grant Nos. 51427801, 11374350, 51201179, and 11274361).
Imaging intracellular protein dynamics by spinning disk confocal microscopy
Stehbens, Samantha; Pemble, Hayley; Murrow, Lindsay; Wittmann, Torsten
2012-01-01
The palette of fluorescent proteins has grown exponentially over the last decade, and as a result live imaging of cells expressing fluorescently tagged proteins is becoming more and more main stream. Spinning disk confocal microscopy (SDC) is a high speed optical sectioning technique, and a method of choice to observe and analyze intracellular fluorescent protein dynamics at high spatial and temporal resolution. In an SDC system, a rapidly rotating pinhole disk generates thousands of points of light that scan the specimen simultaneously, which allows direct capture of the confocal image with low noise scientific grade cooled charged-coupled device (CCD) cameras, and can achieve frame rates of up 1000 frames per second. In this chapter we describe important components of a state-of-the-art spinning disk system optimized for live cell microscopy, and provide a rationale for specific design choices. We also give guidelines how other imaging techniques such as total internal reflection (TIRF) microscopy or spatially controlled photoactivation can be coupled with SDC imaging, and provide a short protocol on how to generate cell lines stably expressing fluorescently tagged proteins by lentivirus-mediated transduction. PMID:22264541
Spin dynamics in relativistic light-matter interaction
NASA Astrophysics Data System (ADS)
Bauke, Heiko; Ahrens, Sven; Keitel, Christoph H.; Grobe, Rainer
2015-05-01
Various spin effects are expected to become observable in light-matter interaction at relativistic intensities. Relativistic quantum mechanics equipped with a suitable relativistic spin operator forms the theoretical foundation for describing these effects. Various proposals for relativistic spin operators have been offered by different authors, which are presented in a unified way. As a result of the operators' mathematical properties only the Foldy-Wouthuysen operator and the Pryce operator qualify as possible proper relativistic spin operators. The ground states of highly charged hydrogen-like ions can be utilized to identify a legitimate relativistic spin operator experimentally. Subsequently, the Foldy-Wouthuysen spin operator is employed to study electron-spin precession in high-intensity standing light waves with elliptical polarization. For a correct theoretical description of the predicted electron-spin precession relativistic effects due to the spin angular momentum of the electromagnetic wave has to be taken into account even in the limit of low intensities.
Jungfleisch, Matthias B.; Zhang, Wei; Jiang, Wanjun; Sklenar, Joseph; Pearson, John E.; Ketterson, John B.; Hoffmann, Axel
2016-01-01
The understanding of spin dynamics in laterally confined structures on sub-micron length scales has become a significant aspect of the development of novel magnetic storage technologies. Numerous ferromagnetic resonance measurements, optical characterization by Kerr microscopy and Brillouin light scattering spectroscopy and x-ray studies were carried out to detect the dynamics in patterned magnetic antidot lattices. Here, we investigate Oersted-field driven spin dynamics in rectangular Ni80Fe20/Pt antidot lattices with different lattice parameters by electrical means. When the system is driven to resonance, a dc voltage across the length of the sample is detected that changes its sign upon field reversal, which is in agreement with a rectification mechanism based on the inverse spin Hall effect. Furthermore, we show that the voltage output scales linearly with the applied microwave drive in the investigated range of powers. Our findings have direct implications on the development of engineered magnonics applications and devices.
Spinning Black Hole Pairs: Dynamics and Gravitational Waves
NASA Astrophysics Data System (ADS)
Grossman, Rebecca
Black hole binaries will be an important source of gravitational radiation for both ground-based and future space-based gravitational wave detectors. The study of such systems will offer a unique opportunity to test the dynamical predictions of general relativity when gravity is very strong. To date, most investigations of black hole binary dynamics have focused attention on restricted scenarios in which the black holes do not spin (and thus are confined to move in a plane) and/or in which they stay on quasi-circular orbits. However, spinning black hole pairs in eccentric orbits are now understood to be astrophysically equally important. These spinning binaries exhibit a range of complicated dynamical behaviors, even in the absence of radiation reaction. Their conservative dynamics is complicated by extreme perihelion precession compounded by spin-induced precession. Although the motion seems to defy simple decoding, we are able to quantitatively define and describe the fully three-dimensional motion of arbitrary mass-ratio binaries with at least one black hole spinning and expose an underlying simplicity. To do so, we untangle the dynamics by constructing an instantaneous orbital plane and showing that the motion captured in that plane obeys elegant topological rules. In this thesis, we apply the above prescription to two formal systems used to model black hole binaries. The first is defined by the conservative 3PN Hamiltonian plus spin-orbit coupling and is particularly suitable to comparable-mass binaries. The second is defined by geodesics of the Kerr metric and is used exclusively for extreme mass-ratio binaries. In both systems, we define a complete taxonomy for fully three-dimensional orbits. More than just a naming system, the taxonomy provides unambiguous and quantitative descriptions of the orbits, including a determination of the zoom-whirliness of any given orbit. Through a correspondence with the rational numbers, we are able to show that all of the
Meriles, Carlos A.; Doherty, Marcus W.
2014-07-14
Key to future spintronics and spin-based information processing technologies is the generation, manipulation, and detection of spin polarization in a solid state platform. Here, we theoretically explore an alternative route to spin injection via the use of dynamically polarized nitrogen-vacancy (NV) centers in diamond. We focus on the geometry where carriers and NV centers are confined to proximate, parallel layers and use a “trap-and-release” model to calculate the spin cross-relaxation probabilities between the charge carriers and neighboring NV centers. We identify near-unity regimes of carrier polarization depending on the NV spin state, applied magnetic field, and carrier g-factor. In particular, we find that unlike holes, electron spins are distinctively robust against spin-lattice relaxation by other, unpolarized paramagnetic centers. Further, the polarization process is only weakly dependent on the carrier hopping dynamics, which makes this approach potentially applicable over a broad range of temperatures.
Spin dynamics of an individual Cr atom in a semiconductor quantum dot under optical excitation
NASA Astrophysics Data System (ADS)
Lafuente-Sampietro, A.; Utsumi, H.; Boukari, H.; Kuroda, S.; Besombes, L.
2016-08-01
We studied the spin dynamics of a Cr atom incorporated in a II-VI semiconductor quantum dot using photon correlation techniques. We used recently developed singly Cr-doped CdTe/ZnTe quantum dots to access the spin of an individual magnetic atom. Auto-correlation of the photons emitted by the quantum dot under continuous wave optical excitation reveals fluctuations of the localized spin with a timescale in the 10 ns range. Cross-correlation gives quantitative transfer time between Cr spin states. A calculation of the time dependence of the spin levels population in Cr-doped quantum dots shows that the observed spin dynamics is dominated by the exciton-Cr interaction. These measurements also provide a lower bound in the 20 ns range for the intrinsic Cr spin relaxation time.
Dynamics of Spin-Orbit Coupled Bose-Einstein Condensates in a Random Potential
NASA Astrophysics Data System (ADS)
Mardonov, Sh.; Modugno, M.; Sherman, E. Ya.
2015-10-01
Disorder plays a crucial role in spin dynamics in solids and condensed matter systems. We demonstrate that for a spin-orbit coupled Bose-Einstein condensate in a random potential two mechanisms of spin evolution that can be characterized as "precessional" and "anomalous" are at work simultaneously. The precessional mechanism, typical for solids, is due to the condensate displacement. The unconventional anomalous mechanism is due to the spin-dependent velocity producing the distribution of the condensate spin polarization. The condensate expansion is accompanied by a random displacement and fragmentation, where it becomes sparse, as clearly revealed in the spin dynamics. Thus, different stages of the evolution can be characterized by looking at the condensate spin.
Dynamics of Spin-Orbit Coupled Bose-Einstein Condensates in a Random Potential.
Mardonov, Sh; Modugno, M; Sherman, E Ya
2015-10-30
Disorder plays a crucial role in spin dynamics in solids and condensed matter systems. We demonstrate that for a spin-orbit coupled Bose-Einstein condensate in a random potential two mechanisms of spin evolution that can be characterized as "precessional" and "anomalous" are at work simultaneously. The precessional mechanism, typical for solids, is due to the condensate displacement. The unconventional anomalous mechanism is due to the spin-dependent velocity producing the distribution of the condensate spin polarization. The condensate expansion is accompanied by a random displacement and fragmentation, where it becomes sparse, as clearly revealed in the spin dynamics. Thus, different stages of the evolution can be characterized by looking at the condensate spin. PMID:26565441
Polarization propagator approach to the dynamic nuclear electric shielding in LiH molecule
NASA Astrophysics Data System (ADS)
Lazzeretti, P.; Rossi, E.; Zanasi, R.
1983-07-01
The frequency dependence of the dipole electric polarizability and electric shielding tensors of hydrogen and lithium nuclei in the LiH molecule has been studied via some approximations to the polarization propagator method, i.e., STA, TDA, and RPA, allowing for dipole length, velocity, acceleration, and mixed formalisms. The RPA nuclear electric shieldings are in a fairly good agreement with the corresponding experimental data, a discrepancy being observed for the parallel component at the Li nucleus.
Dynamics of two coupled semiconductor spin qubits in a noisy environment
NASA Astrophysics Data System (ADS)
Das Sarma, S.; Throckmorton, Robert E.; Wu, Yang-Le
2016-07-01
We theoretically consider the temporal dynamics of two coupled spin qubits (e.g., semiconductor quantum dots) driven by the interqubit spin-spin coupling. The presence of environmental noise (e.g., charge traps, nuclear spins, random magnetic impurities) is accounted for by including random magnetic field and random interqubit coupling terms in the Hamiltonian. Both Heisenberg coupling and Ising coupling between the spin qubits are considered, corresponding respectively to exchange and capacitive gates as appropriate for single spin and singlet-triplet semiconductor qubit systems, respectively. Both exchange (Heisenberg) and capacitive (Ising) coupling situations can be solved numerically exactly even in the presence of noise, leading to the key findings that (i) the steady-state return probability to the initial state remains close to unity in the presence of strong noise for many, but not all, starting spin configurations, and (ii) the return probability as a function of time is oscillatory with a characteristic noise-controlled decay toward the steady-state value. We also provide results for the magnetization dynamics of the coupled two-qubit system. Our predicted dynamics can be directly tested in the already existing semiconductor spin qubit setups providing insight into their coherent interaction dynamics. Retention of the initial state spin memory even in the presence of strong environmental noise has important implications for quantum computation using spin qubits.
Probing ultrafast spin dynamics with optical pump-probe scanning tunnelling microscopy.
Yoshida, Shoji; Aizawa, Yuta; Wang, Zi-han; Oshima, Ryuji; Mera, Yutaka; Matsuyama, Eiji; Oigawa, Haruhiro; Takeuchi, Osamu; Shigekawa, Hidemi
2014-08-01
Studies of spin dynamics in low-dimensional systems are important from both fundamental and practical points of view. Spin-polarized scanning tunnelling microscopy allows localized spin dynamics to be characterized and plays important roles in nanoscale science and technology. However, nanoscale analysis of the ultrafast dynamics of itinerant magnetism, as well as its localized characteristics, should be pursued to advance further the investigation of quantum dynamics in functional structures of small systems. Here, we demonstrate the optical pump-probe scanning tunnelling microscopy technique, which enables the nanoscale probing of spin dynamics with the temporal resolution corresponding, in principle, to the optical pulse width. Spins are optically oriented using circularly polarized light, and their dynamics are probed by scanning tunnelling microscopy based on the optical pump-probe method. Spin relaxation in a single quantum well with a width of 6 nm was observed with a spatial resolution of ∼ 1 nm. In addition to spin relaxation dynamics, spin precession, which provides an estimation of the Landé g factor, was observed successfully. PMID:24974938
Probing ultrafast spin dynamics with optical pump-probe scanning tunnelling microscopy
NASA Astrophysics Data System (ADS)
Yoshida, Shoji; Aizawa, Yuta; Wang, Zi-Han; Oshima, Ryuji; Mera, Yutaka; Matsuyama, Eiji; Oigawa, Haruhiro; Takeuchi, Osamu; Shigekawa, Hidemi
2014-08-01
Studies of spin dynamics in low-dimensional systems are important from both fundamental and practical points of view. Spin-polarized scanning tunnelling microscopy allows localized spin dynamics to be characterized and plays important roles in nanoscale science and technology. However, nanoscale analysis of the ultrafast dynamics of itinerant magnetism, as well as its localized characteristics, should be pursued to advance further the investigation of quantum dynamics in functional structures of small systems. Here, we demonstrate the optical pump-probe scanning tunnelling microscopy technique, which enables the nanoscale probing of spin dynamics with the temporal resolution corresponding, in principle, to the optical pulse width. Spins are optically oriented using circularly polarized light, and their dynamics are probed by scanning tunnelling microscopy based on the optical pump-probe method. Spin relaxation in a single quantum well with a width of 6 nm was observed with a spatial resolution of ~1 nm. In addition to spin relaxation dynamics, spin precession, which provides an estimation of the Landé g factor, was observed successfully.
Dynamical theory of spin noise and relaxation: Prospects for real-time NMR measurements.
Field, Timothy R
2014-11-01
Recent developments in theoretical aspects of spin noise and relaxation and their interrelationship reveal a modified spin density, distinct from the density matrix, as the necessary object to describe fluctuations in spin systems. These fluctuations are to be viewed as an intrinsic quantum mechanical property of such systems immersed in random magnetic environments and are observed as "spin noise" in the absence of any radio frequency excitation. With the prospect of ultrafast digitization, the role of spin noise in real-time parameter extraction for (NMR) spin systems, and the advantage over standard techniques, is of essential importance, especially for systems containing a small number of spins. In this article we outline prospects for harnessing the recent dynamical theory in terms of spin-noise measurement, with attention to real-time properties. PMID:25493776
Electrical manipulation of dynamic magnetic impurity and spin texture of helical Dirac fermions
NASA Astrophysics Data System (ADS)
Wang, Rui-Qiang; Zhong, Min; Zheng, Shi-Han; Yang, Mou; Wang, Guang-Hui
2016-05-01
We have theoretically investigated the spin inelastic scattering of helical electrons off a high-spin nanomagnet absorbed on a topological surface. The nanomagnet is treated as a dynamic quantum spin and driven by the spin transfer torque effect. We proposed a mechanism to electrically manipulate the spin texture of helical Dirac fermions rather than by an external magnetic field. By tuning the bias voltage and the direction of impurity magnetization, we present rich patterns of spin texture, from which important fingerprints exclusively associated with the spin helical feature are obtained. Furthermore, it is found that the nonmagnetic potential can create the resonance state in the spin density with different physics as the previously reported resonance of charge density.
Sezer, Deniz; Freed, Jack H; Roux, Benoit
2008-09-01
Simulating electron spin resonance (ESR) spectra directly from molecular dynamics simulations of a spin-labeled protein necessitates a large number (hundreds or thousands) of relatively long (hundreds of nanoseconds) trajectories. To meet this challenge, we explore the possibility of constructing accurate stochastic models of the spin label dynamics from atomistic trajectories. A systematic, two-step procedure, based on the probabilistic framework of hidden Markov models, is developed to build a discrete-time Markov chain process that faithfully captures the internal spin label dynamics on time scales longer than about 150 ps. The constructed Markov model is used both to gain insight into the long-lived conformations of the spin label and to generate the stochastic trajectories required for the simulation of ESR spectra. The methodology is illustrated with an application to the case of a spin-labeled poly alanine alpha helix in explicit solvent. PMID:18698714
Demissie, Taye Beyene
2016-01-28
The nuclear spin-rotation (NSR) and absolute nuclear magnetic resonance (NMR) shielding tensors of the nuclei in the series of X(77)Se and X(125)Te (X = (29)Si, (73)Ge, (119)Sn and (207)Pb) are calculated using four-component relativistic density functional theory (DFT) and coupled-cluster singles-doubles with a perturbative triples correction (CCSD(T)). The results for the NSR constants are compared to available experimental data. The best theoretical estimates are obtained when relativistic corrections from DFT are added to the accurate non-relativistic CCSD(T) results. All the calculated NSR constants are in excellent agreement with the corresponding experimental values. Even though there are previously estimated absolute shielding constants and spans from experimental NSR tensors, new accurate values are reported following the same approach used to calculate the NSR constants in this study. The main reasons for the discrepancy between the previously reported NMR properties and the accurate results obtained in this study are also discussed. PMID:26741559
Measurement backaction on the quantum spin-mixing dynamics of a spin-1 Bose-Einstein condensate
Zhang Keye; Zhou Lu; Zhang Weiping; Ling, Hong Y.; Pu Han
2011-06-15
We consider a small F=1 spinor condensate inside an optical cavity driven by an optical probe field, and subject the output of the probe to a homodyne detection, with the goal of investigating the effect of measurement backaction on the spin dynamics of the condensate. Using the stochastic master equation approach, we show that the effect of backaction is sensitive to not only the measurement strength but also the quantum fluctuation of the spinor condensate. The same method is also used to estimate the atom numbers below which the effect of backaction becomes so prominent that extracting spin dynamics from this cavity-based detection scheme is no longer practical.
Dynamics of domain wall driven by spin-transfer torque
Chureemart, P.; Evans, R. F. L.; Chantrell, R. W.
2011-05-01
Spin-torque switching of magnetic devices offers new technological possibilities for data storage and integrated circuits. We have investigated domain-wall motion in a ferromagnetic thin film driven by a spin-polarized current using an atomistic spin model with a modified Landau-Lifshitz-Gilbert equation including the effect of the spin-transfer torque. The presence of the spin-transfer torque is shown to create an out-of-plane domain wall, in contrast to the external-field-driven case where an in-plane wall is found. We have investigated the effect of the spin torque on domain-wall displacement, domain-wall velocity, and domain-wall width, as well as the equilibration time in the presence of the spin-transfer torque. We have shown that the minimum spin-current density, regarded as the critical value for domain-wall motion, decreases with increasing temperature.
Signature of magnetization dynamics in spin-transfer-driven nanopillars with tilted easy axis
NASA Astrophysics Data System (ADS)
Zhang, Hong; Lin, Weiwei; Mangin, Stéphane; Zhang, Zongzhi; Liu, Yaowen
2013-01-01
Special spin-transfer-driven magnetic behaviors can take place in a spin valve nanopillar with perpendicular anisotropy due to reduced symmetry of easy axis. Micromagnetic simulation demonstrates a dip in the average magnetization curve, which corresponds to the experimentally observed undulation of dc resistance. The dip is a signature of spin-transfer-driven reversable magnetic process with slightly tilted easy axis in the free layer. This featured magnetization dynamics includes non-uniform magnetization precession and multi-mode propagating spin waves, which are attributed to the competition among tilted magnetic anisotropy, magnetic field, and spin transfer torque.
Dynamical self-quenching of spin pumping into double quantum dots.
Brataas, Arne; Rashba, Emmanuel I
2012-12-01
Nuclear spin polarization can be pumped into spin-blockaded quantum dots by multiple Landau-Zener passages through singlet-triplet anticrossings. By numerical simulations of realistic systems with 10(7) nuclear spins during 10(5) sweeps, we uncover a mechanism of dynamical self-quenching which results in a fast saturation of the nuclear polarization under stationary pumping. This is caused by screening the random field of the nuclear spins. For moderate spin-orbit coupling, self-quenching persists but its patterns are modified. Our finding explains low polarization levels achieved experimentally and calls for developing new protocols that break the self-quenching limitations. PMID:23368239
Low-energy-state dynamics of entanglement for spin systems
Jafari, R.
2010-11-15
We develop the ideas of the quantum renormalization group and quantum information by exploring the low-energy-state dynamics of entanglement resources of a system close to its quantum critical point. We demonstrate that low-energy-state dynamical quantities of one-dimensional magnetic systems can show a quantum phase transition point and show scaling behavior in the vicinity of the transition point. To present our idea, we study the evolution of two spin entanglements in the one-dimensional Ising model in the transverse field. The system is initialized as the so-called thermal ground state of the pure Ising model. We investigate the evolution of the generation of entanglement with increasing magnetic field. We obtain that the derivative of the time at which the entanglement reaches its maximum with respect to the transverse field diverges at the critical point and its scaling behaviors versus the size of the system are the same as the static ground-state entanglement of the system.
Free vibration and dynamic response analysis of spinning structures
NASA Technical Reports Server (NTRS)
1986-01-01
The proposed effort involved development of numerical procedures for efficient solution of free vibration problems of spinning structures. An eigenproblem solution procedure, based on a Lanczos method employing complex arithmetic, was successfully developed. This task involved formulation of the numerical procedure, FORTRAN coding of the algorithm, checking and debugging of software, and implementation of the routine in the STARS program. A graphics package for the E/S PS 300 as well as for the Tektronix terminals was successfully generated and consists of the following special capabilities: (1) a dynamic response plot for the stresses and displacements as functions of time; and (2) a menu driven command module enabling input of data on an interactive basis. Finally, the STARS analysis capability was further improved by implementing the dynamic response analysis package that provides information on nodal deformations and element stresses as a function of time. A number of test cases were run utilizing the currently developed algorithm implemented in the STARS program and such results indicate that the newly generated solution technique is significantly more efficient than other existing similar procedures.
Self-Polarization and Dynamical Cooling of Nuclear Spins in Double Quantum Dots
NASA Astrophysics Data System (ADS)
Rudner, M. S.; Levitov, L. S.
2007-07-01
The spin-blockade regime of double quantum dots features coupled dynamics of electron and nuclear spins resulting from the hyperfine interaction. We explain observed nuclear self-polarization via a mechanism based on feedback of the Overhauser shift on electron energy levels, and propose to use the instability toward self-polarization as a vehicle for controlling the nuclear spin distribution. In the dynamics induced by a properly chosen time-dependent magnetic field, nuclear spin fluctuations can be suppressed significantly below the thermal level.
On the accuracy of the state space restriction approximation for spin dynamics simulations
NASA Astrophysics Data System (ADS)
Karabanov, Alexander; Kuprov, Ilya; Charnock, G. T. P.; van der Drift, Anniek; Edwards, Luke J.; Köckenberger, Walter
2011-08-01
We present an algebraic foundation for the state space restriction approximation in spin dynamics simulations and derive applicability criteria as well as minimal basis set requirements for practically encountered simulation tasks. The results are illustrated with nuclear magnetic resonance (NMR), electron spin resonance (ESR), dynamic nuclear polarization (DNP), and spin chemistry simulations. It is demonstrated that state space restriction yields accurate results in systems where the time scale of spin relaxation processes approximately matches the time scale of the experiment. Rigorous error bounds and basis set requirements are derived.
Dynamical decoupling design for identifying weakly coupled nuclear spins in a bath
NASA Astrophysics Data System (ADS)
Zhao, Nan; Wrachtrup, Jörg; Liu, Ren-Bao
2014-09-01
Identifying weakly coupled nuclear spins around single electron spins is a key step toward implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single-spin nuclear magnetic resonance detection using diamond defect spins. Dynamical decoupling control of the center electron spin with periodic pulse sequences [e.g., the Carre-Purcell-Meiboom-Gill (CPMG) sequence] has been successfully used to identify single nuclear spins and to resolve structure of nuclear spin clusters. Here, we design a type of pulse sequence by replacing the repetition unit (a single π pulse) of the CPMG sequence with a group of nonuniformly spaced π pulses. Using the nitrogen-vacancy center system in diamond, we theoretically demonstrate that the designed pulse sequence improves the resolution of nuclear spin noise spectroscopy, and more information about the surrounding nuclear spins is extracted. The principle of dynamical decoupling design proposed in this paper is useful in many systems (e.g., defect spin qubit in solids, trapped ion, and superconducting qubit) for high-resolution noise spectroscopy.
Assessing intracranial vascular compliance using dynamic arterial spin labeling.
Yan, Lirong; Liu, Collin Y; Smith, Robert X; Jog, Mayank; Langham, Michael; Krasileva, Kate; Chen, Yufen; Ringman, John M; Wang, Danny J J
2016-01-01
Vascular compliance (VC) is an important marker for a number of cardiovascular diseases and dementia, which is typically assessed in the central and peripheral arteries indirectly by quantifying pulse wave velocity (PWV), and/or pulse pressure waveform. To date, very few methods are available for the quantification of intracranial VC. In the present study, a novel MRI technique for in-vivo assessment of intracranial VC was introduced, where dynamic arterial spin labeling (ASL) scans were synchronized with the systolic and diastolic phases of the cardiac cycle. VC is defined as the ratio of change in arterial cerebral blood volume (ΔCBV) and change in arterial pressure (ΔBP). Intracranial VC was assessed in different vascular components using the proposed dynamic ASL method. Our results show that VC mainly occurs in large arteries, and gradually decreases in small arteries and arterioles. The comparison of intracranial VC between young and elderly subjects shows that aging is accompanied by a reduction of intracranial VC, in good agreement with the literature. Furthermore, a positive association between intracranial VC and cerebral perfusion measured using pseudo-continuous ASL with 3D GRASE MRI was observed independent of aging effects, suggesting loss of VC is associated with a decline in perfusion. Finally, a significant positive correlation between intracranial and central (aortic arch) VC was observed using an ungated phase-contrast 1D projection PWV technique. The proposed dynamic ASL method offers a promising approach for assessing intracranial VC in a range of cardiovascular diseases and dementia. PMID:26364865
Dynamics of the collective modes of an inhomogeneous spin ensemble in a cavity
Wesenberg, Janus H.; Kurucz, Zoltan; Moelmer, Klaus
2011-02-15
We study the excitation dynamics of an inhomogeneously broadened spin ensemble coupled to a single cavity mode. The collective excitations of the spin ensemble can be described in terms of generalized spin waves, and, in the absence of the cavity, the free evolution of the spin ensemble can be described as a drift in the wavenumber without dispersion. In this article we show that the dynamics in the presence of coupling to the cavity mode can be described solely by a modified time evolution of the wavenumbers. In particular, we show that collective excitations with a well-defined wavenumber pass without dispersion from negative to positive-valued wavenumbers without populating the zero wavenumber spin wave mode. The results are relevant for multimode collective quantum memories where qubits are encoded in different spin waves.
Relaxation and coherent oscillations in the spin dynamics of II-VI diluted magnetic quantum wells
NASA Astrophysics Data System (ADS)
Ungar, F.; Cygorek, M.; Tamborenea, P. I.; Axt, V. M.
2015-10-01
We study theoretically the ultrafast spin dynamics of II-VI diluted magnetic quantum wells in the presence of spin-orbit interaction. We extend a recent study where it was shown that the spin-orbit interaction and the exchange sd coupling in bulk and quantum wells can compete resulting in qualitatively new dynamics when they act simultaneously. We concentrate on Hg1-x-yMnxCdyTe quantum wells, which have a highly tunable Rashba spin-orbit coupling. Our calculations use a recently developed formalism which incorporates electronic correlations originating from the exchange sd-coupling. We find that the dependence of electronic spin oscillations on the excess energy changes qualitatively depending on whether or not the spin-orbit interaction dominates or is of comparable strength with the sd interaction.
Control of spin dynamics in a two-dimensional electron gas by electromagnetic dressing
NASA Astrophysics Data System (ADS)
Pervishko, A. A.; Kibis, O. V.; Morina, S.; Shelykh, I. A.
2015-11-01
We solved the Schrödinger problem for a two-dimensional electron gas (2DEG) with the Rashba spin-orbit interaction in the presence of a strong high-frequency electromagnetic field (dressing field). The found eigenfunctions and eigenenergies of the problem are used to describe the spin dynamics of the dressed 2DEG within the formalism of the density matrix response function. Solving the equations of spin dynamics, we show that the dressing field can switch the spin relaxation in the 2DEG between the cases corresponding to the known Elliott-Yafet and D'yakonov-Perel' regimes. As a result, the spin properties of the 2DEG can be tuned by a high-frequency electromagnetic field. The present effect opens an unexplored way for controlling the spin with light and, therefore, forms the physical prerequisites for creating light-tuned spintronics devices.
Spinach - A software library for simulation of spin dynamics in large spin systems
NASA Astrophysics Data System (ADS)
Hogben, H. J.; Krzystyniak, M.; Charnock, G. T. P.; Hore, P. J.; Kuprov, Ilya
2011-02-01
We introduce a software library incorporating our recent research into efficient simulation algorithms for large spin systems. Liouville space simulations (including symmetry, relaxation and chemical kinetics) of most liquid-state NMR experiments on 40+ spin systems can now be performed without effort on a desktop workstation. Much progress has also been made with improving the efficiency of ESR, solid state NMR and Spin Chemistry simulations. Spinach is available for download at http://spindynamics.org.
Observation of Dynamical spin shielding in Ce: Why It Matters for Pu Electronic Structure
Tobin, J G; Yu, S W; Chung, B W; Morton, S A; Komesua, T; Waddill, G D
2007-03-08
In a series of experiments and linked theoretical modeling, the range of possible solutions for Pu electronic structure has been dramatically reduced. Nevertheless, the key issue of electron correlation remains.
Self-consistent description of spin-phonon dynamics in ferromagnets
NASA Astrophysics Data System (ADS)
Nieves, P.; Serantes, D.; Chubykalo-Fesenko, O.
2016-07-01
Several recently reported exciting phenomena such as spin caloritronics or ultrafast laser-induced spin dynamics involve the action of temperature on spin dynamics. However, the inverse effect of magnetization dynamics on temperature change is very frequently ignored. Based on the density matrix approach, in this work we derive a self-consistent model for describing the magnetization and phonon temperature dynamics in ferromagnets in the framework of the quantum Landau-Lifshitz-Bloch equation. We explore potential applicability of our approach for two cases, inspired by magnetocaloric effect and magnetic fluid hyperthermia. In the first case, the spin-phonon dynamics is governed by the longitudinal relaxation in bulk systems close to the Curie temperature; while in the second case it is described by the transverse relaxation during the hysteresis cycle of individual nanoparticles well below the Curie temperature.
Dynamic Structure Factors of the Spin-1/2 XX Chain with Dzyaloshinskii-Moriya Interaction
NASA Astrophysics Data System (ADS)
Derzhko, Oleg; Verkholyak, Taras
2006-10-01
We consider the spin-1/2 isotropic XY chain in a (z) transverse magnetic field with the Dzyaloshinskii-Moriya interaction directed along the z-axis in spin space and examine the effects of the latter interaction on the zz, xx (yy) and xy (yx) dynamic structure factors. The Dzyaloshinskii-Moriya interaction does not manifest itself in the zz dynamic quantities. In contrast, the xx (yy) and xy (yx) dynamic structure factors show dramatical changes owing to the Dzyaloshinskii-Moriya interaction. Implications of our results for electron spin resonance experiments are briefly discussed.
Electron-Nuclear Spin Dynamics in a Mesoscopic Solid-State Quantum Computer
Berman, G.P.; Campbell, D.K.; Doolen, G.D.; Nagaev, K.E.
1998-12-07
We numerically simulate the process of nuclear spin measurement in Kane's quantum computer. For this purpose, we model the quantum dynamics of two coupled nuclear spins located on {sup 31}P donors implanted in Si. We estimate the minimum time of measurement necessary for the reliable transfer of quantum information from the nuclear spin subsystem to the electronic one and the probability of error for typical values of external noise.
Spin echo dynamics under an applied drift field in graphene nanoribbon superlattices
Prabhakar, Sanjay; Melnik, Roderick; Bonilla, Luis L.; Raynolds, James E.
2013-12-02
We investigate the evolution of spin dynamics in graphene nanoribbon superlattices (GNSLs) with armchair and zigzag edges in the presence of a drift field. We determine the exact evolution operator and show that it exhibits spin echo phenomena due to rapid oscillations of the quantum states along the ribbon. The evolution of the spin polarization is accompanied by strong beating patterns. We also provide detailed analysis of the band structure of GNSLs with armchair and zigzag edges.
Nonlinear analysis of magnetization dynamics excited by spin Hall effect
NASA Astrophysics Data System (ADS)
Taniguchi, Tomohiro
2015-03-01
We investigate the possibility of exciting self-oscillation in a perpendicular ferromagnet by the spin Hall effect on the basis of a nonlinear analysis of the Landau-Lifshitz-Gilbert (LLG) equation. In the self-oscillation state, the energy supplied by the spin torque during a precession on a constant energy curve should equal the dissipation due to damping. Also, the current to balance the spin torque and the damping torque in the self-oscillation state should be larger than the critical current to destabilize the initial state. We find that these conditions in the spin Hall system are not satisfied by deriving analytical solutions of the energy supplied by the spin transfer effect and the dissipation due to the damping from the nonlinear LLG equation. This indicates that the self-oscillation of a perpendicular ferromagnet cannot be excited solely by the spin Hall torque.
Detection and Measurement of Spin-Dependent Dynamics in Random Telegraph Signals
NASA Astrophysics Data System (ADS)
House, M. G.; Xiao, Ming; Guo, GuoPing; Li, HaiOu; Cao, Gang; Rosenthal, M. M.; Jiang, HongWen
2013-09-01
A quantum point contact was used to observe single-electron fluctuations of a quantum dot in a GaAs heterostructure. The resulting random telegraph signals (RTS) contain statistical information about the electron spin state if the tunneling dynamics are spin dependent. We develop a statistical method to extract information about spin-dependent dynamics from RTS and use it to demonstrate that these dynamics can be studied in the thermal energy regime. The tunneling rates of each spin state are independently measured in a finite external magnetic field. We confirm previous findings of a decrease in overall tunneling rates for the spin excited state compared to the ground state as an external magnetic field is increased.
Uncovering the features of spin dynamics in hadronic physics
NASA Astrophysics Data System (ADS)
Goldstein, G. R.; Arash, F.
1990-06-01
We summarize the program pursued by Michael J. Moravcsik and the authors on spin amplitude analyses and interpretation. We present the recent observations that “phase histograms” reveal striking peaks corresponding to spin amplitudes that tend to have definite simple phase relations. An interpretation is proposed in which the spin amplitudes receive a coherent and an incoherent contribution over large ranges of energies and angles. Continuing research directions are reported.
Decoherence induced by a dynamic spin environment: The universal regime
Cormick, Cecilia; Paz, Juan Pablo
2008-02-15
This paper analyzes the decoherence induced on a single qubit by the interaction with a spin chain with nontrivial internal dynamics (XY-type interactions). The aim of the paper is to study the existence and properties of the so-called universal regime, in which the decoherence time scale becomes independent of the strength of the coupling with the environment. It is shown that, although such a regime does exist, as previously established by Cucchietti et al. [Phys. Rev. A 75, 032337 (2007)], it is not a clear signature of a quantum phase transition in the environment. In fact, this kind of universality also exists in the absence of quantum phase transitions. A universal regime can be related to the existence of an energy scale separation between the Hamiltonian of the environment and the one characterizing the system-environment interaction. The results presented also indicate that in the strong-coupling regime the quantum phase transition does not produce an enhancement of decoherence (as opposed to what happens in the weak-coupling regime)
Charge and Spin Dynamics of the Hubbard Chains
NASA Technical Reports Server (NTRS)
Park, Youngho; Liang, Shoudan
1999-01-01
We calculate the local correlation functions of charge and spin for the one-chain and two-chain Hubbard model using density matrix renormalization group method and the recursion technique. Keeping only finite number of states we get good accuracy for the low energy excitations. We study the charge and spin gaps, bandwidths and weights of the spectra for various values of the on-site Coulomb interaction U and the electron filling. In the low energy part, the local correlation functions are different for the charge and spin. The bandwidths are proportional to t for the charge and J for the spin respectively.
Next-to-leading order gravitational spin(1)-spin(2) dynamics in Hamiltonian form
Steinhoff, Jan; Hergt, Steven; Schaefer, Gerhard
2008-04-15
Based on recent developments by the authors a next-to-leading order spin(1)-spin(2) Hamiltonian is derived for the first time. The result is obtained within the canonical formalism of Arnowitt, Deser, and Misner (ADM) utilizing their generalized isotropic coordinates. A comparison with other methods is given.
Reading charge transport from the spin dynamics on the surface of a topological insulator.
Liu, Xin; Sinova, Jairo
2013-10-18
Resolving the conductance of the topological surface states (TSSs) from the bulk contribution has been a great challenge for studying the transport properties of topological insulators. By developing a nonperturbative diffusion equation that describes fully the spin-charge dynamics in the strong spin-orbit coupling regime, we present a proposal to read the charge transport information of TSSs from its spin dynamics which can be isolated from the bulk contribution by the time-resolved second harmonic generation pump-probe measurement. We demonstrate the qualitatively different Dyaknov-Perel spin relaxation behavior between the TSSs and the two-dimensional spin-orbit coupling electron gas. The decay time of both in-plane and out-of-plane spin polarization is naturally proved to be identical to the charge transport time. The out-of-plane spin dynamics is shown to be in the experimentally reachable regime of the femtosecond pump-probe spectroscopy and thereby we suggest experiments to detect the charge transport properties of the TSSs from their unique spin dynamics. PMID:24182290
Quantum phases and dynamics of geometric phase in a quantum spin chain under linear quench
NASA Astrophysics Data System (ADS)
Sarkar, S.; Basu, B.
2012-12-01
We study the quantum phases of anisotropic XY spin chain in presence and absence of adiabatic quench. A connection between geometric phase and criticality is established from the dynamical behavior of the geometric phase for a quench induced quantum phase transition in a quantum spin chain. We predict XX criticality associated with a sequence of non-contractible geometric phases.
Effect of electron electric dipole moment on the spin dynamics of the YbF molecule
NASA Astrophysics Data System (ADS)
Soga, Kota; Fukuda, Masahiro; Senami, Masato; Tachibana, Akitomo
2014-09-01
The existence of the large value of the electron electric dipole moment (EDM) is predicted in extensions of the standard model (SM). To find or exclude physics beyond SM, the EDM is studied in many experiments, where the precession motion of the electron spin is used for the detection. This motion depends on the internal effective electric field (EEF). The accurate prediction of the relation between the EDM and the spin motion is mandatory for deriving the constraint of the EDM. In addition to the computation of EEF, our group studies the spin dynamics by the equation of motion (EOM) of spin. In our group, we have studied the spin motion based on quantum field theory (QFT). In QFT, the spin motion is governed by the spin torque and zeta force. The latter gives local effects and cannot be described in quantum mechanics (QM). Hence, in our approach, there is a difference from ordinary treatment of the spin motion based on QM. In this work, we show that the existence of the EDM modifies our EOM of the spin, that is, the EDM gives the additional contribution to the spin torque. This torque is induced by not only electric field but also magnetic field as a result of relativistic generalization. Then we show our results of the local spin torque distribution for the YbF molecule.
Spin transport and dynamics in the F/N junction
NASA Astrophysics Data System (ADS)
Li, Hua; Bedell, Kevin
2015-03-01
We study the spin transport in the low temperature regime (often referred to as the precession-dominated regime) between a ferromagnetic Fermi liquid (FFL) and a normal metal metallic Fermi liquid (NFL), the F/N junction, which is considered one of the basic spintronic devices. In particular, we explore the propagation of spin waves and transport of magnetization through the interface of the F/N junction where non-equilibrium spin polarization is created on the normal metal side of the junction by spin injection. We calculate the probable spin wave modes in the precession-dominated regime on both sides of the junction especially on the NFL side where the system is out of equilibrium. Proper boundary conditions at the interface are introduced to establish the transport of the spin properties through the F/N junction. In the end, a possible transmission conduction electron spin resonance experiment is suggested on the F/N junction to see if the predicted spin wave modes could propagate through the junction.
Effects of ruthenium seed layer on the microstructure and spin dynamics of thin permalloy films
NASA Astrophysics Data System (ADS)
Jin, Lichuan; Zhang, Huaiwu; Tang, Xiaoli; Bai, Feiming; Zhong, Zhiyong
2013-02-01
The spin dynamics and microstructure properties of a sputtered 12 nm Ni81Fe19 thin film have been enhanced by the use of a ruthenium seed layer. Both the ferromagnetic resonance field and linewidth are enhanced dramatically as the thickness of ruthenium seed layer is increased. The surface anisotropy energy constant can also be largely tailored from 0.06 to 0.96 erg/cm-2 by changing the seed layer thickness. The changes to the dynamics magnetization properties are caused by both ruthenium seed layer induced changes in the Ni81Fe19 structure properties and surface topography properties. Roughness induced inhomogeneous linewidth broadening is also seen. The damping constant is highly tunable via the ruthenium thickness. This approach can be used to tailor both the structure and spin dynamic properties of thin Ni81Fe19 films over a wide range. And it may benefit the applications of spin dynamics and spin current based devices.
Dynamic neutron scattering on incoherent systems using efficient resonance spin flip techniques
Häussler, Wolfgang; Kredler, Lukas
2014-05-15
We have performed numerical ray-tracing Monte-Carlo-simulations of incoherent dynamic neutron scattering experiments. We intend to optimize the efficiency of incoherent measurements depending on the fraction of neutrons scattered without and with spin flip at the sample. In addition to conventional spin echo, we have numerically and experimentally studied oscillating intensity techniques. The results point out the advantages of these different spin echo variants and are an important prerequisite for neutron resonance spin echo instruments like RESEDA (FRM II, Munich), to choose the most efficient technique depending on the scattering vector range and the properties of the sample system under study.
1H-NMR study of the spin dynamics of fine superparamagnetic nanoparticles
Bordonali, L.; Furukawa, Y.; Kraken, M.; Litterst, F.J.; Sangregorio, C.; Casula, M.F.; Lascialfari, A.
2012-05-25
We report a broadband 1H-NMR study of the temperature spin dynamics of nearly monodisperse dextran-coated γ-Fe2O3 magnetic nanoparticles. We observed a maximum in T1−1(T) that decreases in amplitude and shifts toward higher temperatures with increasing field. We suggest that this is related to the progressive superparamagnetic spin blocking of the ferrite core. The data can be explained by assuming a single electronic spin-spin correlation time and introducing a field-dependent distribution of anisotropy energy barriers.
Spin Crossover in Ferropericlase From First-Principles Molecular Dynamics Simulations
NASA Astrophysics Data System (ADS)
Holmstrom, E.; Stixrude, L. P.
2013-12-01
Ferropericlase is believed to be the second-most abundant mineral of the lower mantle of the Earth. It is experimentally known that with increasing pressure, the iron ions in the mineral begin to collapse from a high-spin to low-spin state. This spin crossover looks certain to have geophysical effects, and hence a good theoretical understanding of the phenomenon is necessary. Using first-principles molecular dynamics simulations in conjunction with thermodynamic integration, we construct a phase diagram of the spin crossover as a function of pressure and temperature. In addition, we predict that the mineral loses its electrically insulating character within the lower mantle.
Magnetization dynamics of topological defects and the spin solid in a kagome artificial spin ice
NASA Astrophysics Data System (ADS)
Bhat, V. S.; Heimbach, F.; Stasinopoulos, I.; Grundler, D.
2016-04-01
We report broadband spin-wave spectroscopy on kagome artificial spin ice (ASI) made of large arrays of interconnected Ni80Fe20 nanobars. Spectra taken in saturated and disordered states exhibit a series of resonances with characteristic magnetic field dependencies. Making use of micromagnetic simulations, we identify resonances that reflect the spin-solid-state and monopole-antimonopole pairs on Dirac strings. The latter resonances allow for the generation of highly charged vertices in ASIs via microwave-assisted switching. Our findings open further perspectives for fundamental studies on ASIs and their usage in reprogrammable magnonics.
Lattice Dynamics of EuO: Evidence for Giant Spin-Phonon Coupling
NASA Astrophysics Data System (ADS)
Pradip, R.; Piekarz, P.; Bosak, A.; Merkel, D. G.; Waller, O.; Seiler, A.; Chumakov, A. I.; Rüffer, R.; Oleś, A. M.; Parlinski, K.; Krisch, M.; Baumbach, T.; Stankov, S.
2016-05-01
Comprehensive studies of lattice dynamics in the ferromagnetic semiconductor EuO have been performed by a combination of inelastic x-ray scattering, nuclear inelastic scattering, and ab initio calculations. A remarkably large broadening of the transverse acoustic phonons was discovered at temperatures above and below the Curie temperature TC=69 K . This result indicates a surprisingly strong momentum-dependent spin-phonon coupling induced by the spin dynamics in EuO.
Adelnia, Fatemeh; Lascialfari, Alessandro; Mariani, Manuel; Ammannato, Luca; Caneschi, Andrea; Rovai, Donella; Winpenny, Richard; Timco, Grigore; Corti, Maurizio Borsa, Ferdinando
2015-05-07
We present the room temperature proton nuclear magnetic resonance (NMR) nuclear spin-lattice relaxation rate (NSLR) results in two 1D spin chains: the Heisenberg antiferromagnetic (AFM) Eu(hfac){sub 3}NITEt and the magnetically frustrated Gd(hfac){sub 3}NITEt. The NSLR as a function of external magnetic field can be interpreted very well in terms of high temperature spin dynamics dominated by a long time persistence of the decay of the two-spin correlation function due to the conservation of the total spin value for isotropic Heisenberg chains. The high temperature spin dynamics are also investigated in Heisenberg AFM molecular rings. In both Cr{sub 8} closed ring and in Cr{sub 7}Cd and Cr{sub 8}Zn open rings, i.e., model systems for a finite spin segment, an enhancement of the low frequency spectral density is found consistent with spin diffusion but the high cut-off frequency due to intermolecular anisotropic interactions prevents a detailed analysis of the spin diffusion regime.
Spin dynamics and relaxation in graphene dictated by electron-hole puddles.
Van Tuan, Dinh; Ortmann, Frank; Cummings, Aron W; Soriano, David; Roche, Stephan
2016-01-01
The understanding of spin dynamics and relaxation mechanisms in clean graphene, and the upper time and length scales on which spin devices can operate, are prerequisites to realizing graphene-based spintronic technologies. Here we theoretically reveal the nature of fundamental spin relaxation mechanisms in clean graphene on different substrates with Rashba spin-orbit fields as low as a few tens of μeV. Spin lifetimes ranging from 50 picoseconds up to several nanoseconds are found to be dictated by substrate-induced electron-hole characteristics. A crossover in the spin relaxation mechanism from a Dyakonov-Perel type for SiO2 substrates to a broadening-induced dephasing for hBN substrates is described. The energy dependence of spin lifetimes, their ratio for spins pointing out-of-plane and in-plane, and the scaling with disorder provide a global picture about spin dynamics and relaxation in ultraclean graphene in the presence of electron-hole puddles. PMID:26876333
Probing dynamics of a spin ensemble of P1 centers in diamond using a superconducting resonator
NASA Astrophysics Data System (ADS)
de Lange, Gijs; Ranjan, Vishal; Schutjens, Ron; Debelhoir, Thibault; Groen, Joost; Szombati, Daniel; Thoen, David; Klapwijk, Teun; Hanson, Ronald; Dicarlo, Leonardo
2013-03-01
Solid-state spin ensembles are promising candidates for realizing a quantum memory for superconducting circuits. Understanding the dynamics of such ensembles is a necessary step towards achieving this goal. Here, we investigate the dynamics of an ensemble of nitrogen impurities (P1 centers) in diamond using magnetic-field controlled coupling to the first two modes of a superconducting (NbTiN) coplanar waveguide resonator. Three hyperfine-split spin sub-ensembles are clearly resolved in the 0.25-1.2 K temperature range, with a collective coupling strength extrapolating to 23 MHz at full polarization. The coupling to multiple modes allows us to distinguish the contributions of dipolar broadening and magnetic field inhomogeneity to the spin linewidth. We find the spin polarization recovery rate to be temperature independent below 1 K and conclude that spin out-diffusion across the resonator mode volume provides the mechanism for spin relaxation of the ensemble. Furthermore, by pumping spins in one sub-ensemble and probing the spins in the other sub-ensembles, we observe fast steady-state cross-relaxation (compared to spin repolarization) across the hyperfine transitions. These observations have important implications for using the three sub-ensembles as independent quantum memories. Research supported by NWO, FOM, and EU Project SOLID
Spin dynamics and relaxation in graphene dictated by electron-hole puddles
Van Tuan, Dinh; Ortmann, Frank; Cummings, Aron W.; Soriano, David; Roche, Stephan
2016-01-01
The understanding of spin dynamics and relaxation mechanisms in clean graphene, and the upper time and length scales on which spin devices can operate, are prerequisites to realizing graphene-based spintronic technologies. Here we theoretically reveal the nature of fundamental spin relaxation mechanisms in clean graphene on different substrates with Rashba spin-orbit fields as low as a few tens of μeV. Spin lifetimes ranging from 50 picoseconds up to several nanoseconds are found to be dictated by substrate-induced electron-hole characteristics. A crossover in the spin relaxation mechanism from a Dyakonov-Perel type for SiO2 substrates to a broadening-induced dephasing for hBN substrates is described. The energy dependence of spin lifetimes, their ratio for spins pointing out-of-plane and in-plane, and the scaling with disorder provide a global picture about spin dynamics and relaxation in ultraclean graphene in the presence of electron-hole puddles. PMID:26876333
Spin dynamics and relaxation in graphene dictated by electron-hole puddles
NASA Astrophysics Data System (ADS)
van Tuan, Dinh; Ortmann, Frank; Cummings, Aron W.; Soriano, David; Roche, Stephan
2016-02-01
The understanding of spin dynamics and relaxation mechanisms in clean graphene, and the upper time and length scales on which spin devices can operate, are prerequisites to realizing graphene-based spintronic technologies. Here we theoretically reveal the nature of fundamental spin relaxation mechanisms in clean graphene on different substrates with Rashba spin-orbit fields as low as a few tens of μeV. Spin lifetimes ranging from 50 picoseconds up to several nanoseconds are found to be dictated by substrate-induced electron-hole characteristics. A crossover in the spin relaxation mechanism from a Dyakonov-Perel type for SiO2 substrates to a broadening-induced dephasing for hBN substrates is described. The energy dependence of spin lifetimes, their ratio for spins pointing out-of-plane and in-plane, and the scaling with disorder provide a global picture about spin dynamics and relaxation in ultraclean graphene in the presence of electron-hole puddles.
Dynamical Spin Properties of Confined Fermi and Bose Systems in the Presence of Spin-Orbit Coupling
NASA Astrophysics Data System (ADS)
Ambrosetti, A.; Salasnich, L.; Silvestrelli, P. L.
2016-04-01
Due to the recent experimental progress, tunable spin-orbit (SO) interactions represent ideal candidates for the control of polarization and dynamical spin properties in both quantum wells and cold atomic systems. A detailed understanding of spin properties in SO-coupled systems is thus a compelling prerequisite for possible novel applications or improvements in the context of spintronics and quantum computers. Here, we analyze the case of equal Rashba and Dresselhaus couplings in both homogeneous and laterally confined two-dimensional systems. Starting from the single-particle picture and subsequently introducing two-body interactions we observe that periodic spin fluctuations can be induced and maintained in the system. Through an analytical derivation, we show that the two-body interaction does not involve decoherence effects in the bosonic dimer, and, in the repulsive homogeneous Fermi gas, it may be even exploited in combination with the SO coupling to induce and tune standing currents. By further studying the effects of a harmonic lateral confinement—a particularly interesting case for Bose condensates—we evidence the possible appearance of nontrivial spin textures, whereas the further application of a small Zeeman-type interaction can be exploited to fine-tune the system's polarizability.
NASA Astrophysics Data System (ADS)
Salikhov, R.; Abrudan, R.; Brüssing, F.; Gross, K.; Luo, C.; Westerholt, K.; Zabel, H.; Radu, F.; Garifullin, I. A.
2012-10-01
Using time-resolved x-ray resonant magnetic scattering we report on the precessional dynamics of spin valve systems with parallel (P) and antiparallel (AP) orientation of the ferromagnetic layers separated by a nonmagnetic spacer layers. Previously we observed in Co/Cu/Ni81Fe19(Py) spin valve systems an increase of the magnetic damping parameter in Py with changing magnetization direction of Py and Co layers from P to AP orientation [Salikhov , Appl. Phys. Lett.APPLAB0003-695110.1063/1.3633115 99, 092509 (2011)]. We attributed this finding to the configurational dependence of the spin pumping effect [Kim and Chappert, J. Magn. Magn. Mater.JMMMDC0304-885310.1016/j.jmmm.2004.09.036 286, 56 (2005)]. Here we extend our earlier findings by investigating the temperature dependence of the spin pumping effect and possible other causes for the configurational dependence of the damping parameter, such as domain wall induced coupling or magnetic dipole coupling. The main focus is on Co/Cu/Py trilayers and on Co2MnGe/V/Py trilayers with spin valve properties.
Brownian motion and quantum dynamics of magnetic monopoles in spin ice
Bovo, L.; Bloxsom, J.A.; Prabhakaran, D.; Aeppli, G.; Bramwell, S.T.
2013-01-01
Spin ice illustrates many unusual magnetic properties, including zero point entropy, emergent monopoles and a quasi liquid–gas transition. To reveal the quantum spin dynamics that underpin these phenomena is an experimental challenge. Here we show how crucial information is contained in the frequency dependence of the magnetic susceptibility and in its high frequency or adiabatic limit. The typical response of Dy2Ti2O7 spin ice indicates that monopole diffusion is Brownian but is underpinned by spin tunnelling and is influenced by collective monopole interactions. The adiabatic response reveals evidence of driven monopole plasma oscillations in weak applied field, and unconventional critical behaviour in strong applied field. Our results clarify the origin of the relatively high frequency response in spin ice. They disclose unexpected physics and establish adiabatic susceptibility as a revealing characteristic of exotic spin systems. PMID:23443563
Weyl fermions and spin dynamics of metallic ferromagnet SrRuO3.
Itoh, Shinichi; Endoh, Yasuo; Yokoo, Tetsuya; Ibuka, Soshi; Park, Je-Geun; Kaneko, Yoshio; Takahashi, Kei S; Tokura, Yoshinori; Nagaosa, Naoto
2016-01-01
Weyl fermions that emerge at band crossings in momentum space caused by the spin-orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet. PMID:27273207
Weyl fermions and spin dynamics of metallic ferromagnet SrRuO3
NASA Astrophysics Data System (ADS)
Itoh, Shinichi; Endoh, Yasuo; Yokoo, Tetsuya; Ibuka, Soshi; Park, Je-Geun; Kaneko, Yoshio; Takahashi, Kei S.; Tokura, Yoshinori; Nagaosa, Naoto
2016-06-01
Weyl fermions that emerge at band crossings in momentum space caused by the spin-orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet.
Unified dynamics of electrons and photons via Zitterbewegung and spin-orbit interaction
NASA Astrophysics Data System (ADS)
Leary, C. C.; Smith, Karl H.
2014-02-01
We show that when an electron or photon propagates in a cylindrically symmetric waveguide, it experiences both a Zitterbewegung effect and a spin-orbit interaction leading to identical propagation dynamics for both particles. Applying a unified perturbative approach to both particles simultaneously, we find that to first order in perturbation theory, their Hamiltonians each contain identical Darwin (Zitterbewegung) and spin-orbit terms, resulting in the unification of their dynamics. The presence of the Zitterbewegung effect may be interpreted physically as the delocalization of the electron on the scale of its Compton wavelength, or the delocalization of the photon on the scale of its wavelength in the waveguide. The presence of the spin-orbit interaction leads to the prediction of several rotational effects: the spatial or time evolution of either particle's spin or polarization vector is controlled by the sign of its orbital angular momentum quantum number or, conversely, its spatial wave function is controlled by its spin angular momentum.
Finite temperature spin-dynamics and phase transitions in spin-orbital models
Chen, C.-C.
2010-04-29
We study finite temperature properties of a generic spin-orbital model relevant to transition metal compounds, having coupled quantum Heisenberg-spin and Ising-orbital degrees of freedom. The model system undergoes a phase transition, consistent with that of a 2D Ising model, to an orbitally ordered state at a temperature set by short-range magnetic order. At low temperatures the orbital degrees of freedom freeze-out and the model maps onto a quantum Heisenberg model. The onset of orbital excitations causes a rapid scrambling of the spin spectral weight away from coherent spin-waves, which leads to a sharp increase in uniform magnetic susceptibility just below the phase transition, reminiscent of the observed behavior in the Fe-pnictide materials.
Magnetization dynamics driven by angle-dependent spin-orbit spin-transfer torque
NASA Astrophysics Data System (ADS)
Lee, Seo-Won; Lee, Kyung-Jin
2015-11-01
Spin-orbit torque allows efficient control of the magnetization by using the in-plane current. Recent experiments found a strong angular dependence of spin-orbit torque. We theoretically investigate magnetization switching and domain wall motion induced by an angle-dependent spinorbit torque in perpendicularly magnetized layers. We obtain analytic expressions for the switching current and the domain wall velocity, which are in agreement with numerical results. Based on the expressions, we find that a spin-orbit torque that increases with increasing polar angle of the magnetization is beneficial for both switching and domain wall motion. Our result will serve as a guideline to design and interpret switching and domain wall experiments based on the spin-orbit torque.
NMR measurement of the spin magnetization and spin dynamics in the quantum Hall regimes
NASA Astrophysics Data System (ADS)
Barrett, S. E.; Dabbagh, G.; Pfeiffer, L. N.; West, K. W.; Tycko, R.
1996-07-01
We review our recent measurements of the Knight shift ( Ks( v, T)) and spin-lattice relaxation time ( T1( v,T) of the 71Ga nuclei located in n-doped GaAs quantum wells using optically pumped NMR, for Landau-level filling 0.66 < v < 1.76 and temperature 1.55K< T
SU(2s+1) symmetry and nonlinear dynamics of high spin magnets
Kovalevsky, M.Y. Glushchenko, A.V.
2014-10-15
The article is devoted to the description of dynamics of magnets with arbitrary spin on the basis of the Hamiltonian formalism. The relationship of quantum states and magnetic degrees of freedom has been considered. Subalgebras of Poisson bracket of magnetic values for spin s=1/2; 1; 3/2 have been established. We have obtained non-linear dynamic equations for the normal and degenerate non-equilibrium states of high-spin magnets with the SO(3), SU(4), SU(2)×SU(2), SU(3), SO(4), SO(5) symmetries of exchange interaction. The connection between models of magnetic exchange energy and the Casimir invariants has been discussed.
Probing spin dynamics from the Mott insulating to the superfluid regime in a dipolar lattice gas
NASA Astrophysics Data System (ADS)
de Paz, A.; Pedri, P.; Sharma, A.; Efremov, M.; Naylor, B.; Gorceix, O.; Maréchal, E.; Vernac, L.; Laburthe-Tolra, B.
2016-02-01
We analyze the spin dynamics of an out-of-equilibrium large spin dipolar atomic Bose gas in an optical lattice. We observe a smooth crossover from a complex oscillatory behavior to an exponential behavior throughout the Mott-to-superfluid transition. While both of these regimes are well described by our theoretical models, we provide data in the intermediate regime where dipolar interactions, contact interactions, and superexchange mechanisms compete. In this strongly correlated regime, spin dynamics and transport are coupled, which challenges theoretical models for quantum magnetism.
NASA Astrophysics Data System (ADS)
Podbielski, Jan; Heitmann, Detlef; Grundler, Dirk
2007-11-01
We have studied the spin dynamics of microscopic permalloy rings at GHz frequencies. Increasing the irradiation power, we observe first nonlinear spin dynamics and second microwave-assisted switching (MAS). We explore the MAS phase diagram as a function of microwave power and frequency f and, in particular, extract the critical microwave field hc(f). Its frequency dependence reflects characteristic eigenfrequencies from both the linear and nonlinear spin-wave spectrum. By comparing hc(f) with the different susceptibilities, we gain insight into the microscopic processes which might be the basis of a predictive theory of MAS.
NASA Astrophysics Data System (ADS)
Kaneko, H.; Hada, M.; Nakajima, T.; Nakatsuji, H.
1996-10-01
The 119Sn NMR chemical shifts of SnX 4(X=H, Cl, Br and I) and SnBr 4- nI n ( n = 1, 2, 3) are calculated by the ab initio UHF method including the spin-orbit (SO) interaction combined with the finite perturbation method. The calculated Sn chemical shifts are in good agreement with experiment when the SO interaction is included. As the halogen ligand becomes heavier, the SO effect increases and the chemical shift moves to a higher field. The normal halogen dependence by the substitution from Cl to I in tin tetrahalides is reproduced only when the SO interaction is included. The origin of the SO effect is ascribed to the Fermi contact term.
Formulation of numerical procedures for dynamic analysis of spinning structures
NASA Technical Reports Server (NTRS)
Gupta, K. K.
1986-01-01
The paper presents the descriptions of recently developed numerical algorithms that prove to be useful for the solution of the free vibration problem of spinning structures. First, a generalized procedure for the computation of nodal centrifugal forces in a finite element owing to any specified spin rate is derived in detail. This is followed by a description of an improved eigenproblem solution procedure that proves to be economical for the free vibration analysis of spinning structures. Numerical results are also presented which indicate the efficacy of the currently developed procedures.
Spin dynamics in a quantum point contact showing the 0.7-anomaly
NASA Astrophysics Data System (ADS)
von Delft, Jan; Bauer, Florian; Heyder, Jan; Schimmel, Dennis; CeNS/ASC Team
2015-03-01
The 0.7-anomaly in the first conductance step of a quantum point contact is believed to arise from an interplay of geometry, spin dynamics and interaction effects. Various scenarios have been proposed to explain it, each evoking a different concept, including spontaneous spin polarization, or a quasi-localized state, or ferromagnetic spin fluctuations, or a van Hove ridge (a geometry-induced maximum in the density-of states). Though these scenarios differ substantially regarding numerous details, they all imply anomalous dynamics for the spins in the vicinity of the QPC. We have performed a detailed study of this spin dynamics in the central region of a parabolic quantum point contact, by using the functional renormalization group to calculate the dynamical spin-spin correlation function χ (x ,x' , ω) =∫0∞
Cavity Exciton-Polaritons, Bose Einstein Condensation and Spin Dynamics
Malpuech, Guillaume; Solnyshkov, Dmitry; Shelykh, Ivan
2009-10-07
An introduction giving elementary properties of cavity exciton-polariton will be given. The condition of occurrence of the polariton lasing effect and of the polariton Bose Eintein condensation will be discussed. The impact of the structural disorder on the superfluid behavior of polariton condensates will be analysed. The spin properties of polariton condensates will be discussed. I will show how the anisotropy of the polariton-polariton interaction leads to the suppression of zeeman splitting for polariton condensates (spin Meissner effects). I will show how the combined impact of disorder and spin Meissner effect can lead to the formation of a new condense phase. I will show how these phenomena can allow for the realization of a polaritonic Datta Das spin transistor.
Neutrino spin dynamics in dense matter and electromagnetic field
NASA Astrophysics Data System (ADS)
Arbuzova, E. V.; Lobanov, A. E.; Murchikova, E. M.
2009-01-01
A complete set of solutions to the Dirac-Pauli equation is derived for a massive neutrino that interacts with dense matter and a strong electromagnetic field. It is shown that these solutions may describe neutrino spin precession.
Atom-diatom scattering dynamics of spinning molecules
Eyles, C. J.; Floß, J.; Averbukh, I. Sh.; Leibscher, M.
2015-01-14
We present full quantum mechanical scattering calculations using spinning molecules as target states for nuclear spin selective atom-diatom scattering of reactive D+H{sub 2} and F+H{sub 2} collisions. Molecules can be forced to rotate uni-directionally by chiral trains of short, non-resonant laser pulses, with different nuclear spin isomers rotating in opposite directions. The calculations we present are based on rotational wavepackets that can be created in this manner. As our simulations show, target molecules with opposite sense of rotation are predominantly scattered in opposite directions, opening routes for spatially and quantum state selective scattering of close chemical species. Moreover, two-dimensional state resolved differential cross sections reveal detailed information about the scattering mechanisms, which can be explained to a large degree by a classical vector model for scattering with spinning molecules.
Atom-diatom scattering dynamics of spinning molecules.
Eyles, C J; Floss, J; Averbukh, I Sh; Leibscher, M
2015-01-14
We present full quantum mechanical scattering calculations using spinning molecules as target states for nuclear spin selective atom-diatom scattering of reactive D+H2 and F+H2 collisions. Molecules can be forced to rotate uni-directionally by chiral trains of short, non-resonant laser pulses, with different nuclear spin isomers rotating in opposite directions. The calculations we present are based on rotational wavepackets that can be created in this manner. As our simulations show, target molecules with opposite sense of rotation are predominantly scattered in opposite directions, opening routes for spatially and quantum state selective scattering of close chemical species. Moreover, two-dimensional state resolved differential cross sections reveal detailed information about the scattering mechanisms, which can be explained to a large degree by a classical vector model for scattering with spinning molecules. PMID:25591357
Nuclear magnetometry studies of spin dynamics in quantum Hall systems
NASA Astrophysics Data System (ADS)
Fauzi, M. H.; Watanabe, S.; Hirayama, Y.
2014-12-01
We performed a nuclear magnetometry study on quantum Hall ferromagnet with a bilayer total filling factor of νtot=2 . We found not only a rapid nuclear relaxation but also a sudden change in the nuclear-spin polarization distribution after a one-second interaction with a canted antiferromagnetic phase. We discuss the possibility of observing cooperative phenomena coming from nuclear-spin ensemble triggered by hyperfine interaction in quantum Hall system.
Direct observation of dynamic modes excited in a magnetic insulator by pure spin current.
Demidov, V E; Evelt, M; Bessonov, V; Demokritov, S O; Prieto, J L; Muñoz, M; Ben Youssef, J; Naletov, V V; de Loubens, G; Klein, O; Collet, M; Bortolotti, P; Cros, V; Anane, A
2016-01-01
Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533
Direct observation of dynamic modes excited in a magnetic insulator by pure spin current
Demidov, V. E.; Evelt, M.; Bessonov, V.; Demokritov, S. O.; Prieto, J. L.; Muñoz, M.; Ben Youssef, J.; Naletov, V. V.; de Loubens, G.; Klein, O.; Collet, M.; Bortolotti, P.; Cros, V.; Anane, A.
2016-01-01
Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533
Rényi information flow in the Ising model with single-spin dynamics.
Deng, Zehui; Wu, Jinshan; Guo, Wenan
2014-12-01
The n-index Rényi mutual information and transfer entropies for the two-dimensional kinetic Ising model with arbitrary single-spin dynamics in the thermodynamic limit are derived as functions of ensemble averages of observables and spin-flip probabilities. Cluster Monte Carlo algorithms with different dynamics from the single-spin dynamics are thus applicable to estimate the transfer entropies. By means of Monte Carlo simulations with the Wolff algorithm, we calculate the information flows in the Ising model with the Metropolis dynamics and the Glauber dynamics, respectively. We find that not only the global Rényi transfer entropy, but also the pairwise Rényi transfer entropy, peaks in the disorder phase. PMID:25615223
Rényi information flow in the Ising model with single-spin dynamics
NASA Astrophysics Data System (ADS)
Deng, Zehui; Wu, Jinshan; Guo, Wenan
2014-12-01
The n -index Rényi mutual information and transfer entropies for the two-dimensional kinetic Ising model with arbitrary single-spin dynamics in the thermodynamic limit are derived as functions of ensemble averages of observables and spin-flip probabilities. Cluster Monte Carlo algorithms with different dynamics from the single-spin dynamics are thus applicable to estimate the transfer entropies. By means of Monte Carlo simulations with the Wolff algorithm, we calculate the information flows in the Ising model with the Metropolis dynamics and the Glauber dynamics, respectively. We find that not only the global Rényi transfer entropy, but also the pairwise Rényi transfer entropy, peaks in the disorder phase.
NASA Astrophysics Data System (ADS)
Jungfleisch, Matthias B.; Zhang, Wei; Ding, Junjia; Jiang, Wanjun; Sklenar, Joseph; Pearson, John E.; Ketterson, John B.; Hoffmann, Axel
2016-02-01
The understanding of spin dynamics in laterally confined structures on sub-micron length scales has become a significant aspect of the development of novel magnetic storage technologies. Numerous ferromagnetic resonance measurements, optical characterization by Kerr microscopy and Brillouin light scattering spectroscopy, and x-ray studies were carried out to detect the dynamics in patterned magnetic antidot lattices. Here, we investigate Oersted-field driven spin dynamics in rectangular Ni80Fe20/Pt antidot lattices with different lattice parameters by electrical means and compare them to micromagnetic simulations. When the system is driven to resonance, a dc voltage across the length of the sample is detected that changes its sign upon field reversal, which is in agreement with a rectification mechanism based on the inverse spin Hall effect. Furthermore, we show that the voltage output scales linearly with the applied microwave drive in the investigated range of powers. Our findings have direct implications on the development of engineered magnonics applications and devices.
NASA Astrophysics Data System (ADS)
Carmelo, J. M. P.; Čadež, T.
2016-03-01
A modified version of the metallic-phase pseudofermion dynamical theory (PDT) of the 1D Hubbard model is introduced for the spin dynamical correlation functions of the half-filled 1D Hubbard model Mott-Hubbard phase. The Mott-Hubbard insulator phase PDT is applied to the study of the model longitudinal and transverse spin dynamical structure factors at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. The relation of our theoretical results to both condensed-matter and ultra-cold atom systems is discussed.
Optical initialization and dynamics of spin in a remotely doped quantum well
Kennedy, T. A.; Scheibner, M.; Efros, Al. L.; Bracker, A. S.; Gammon, D.; Shabaev, A.
2006-01-15
The excitation of electron spin polarization and coherence by picosecond light pulses and their dynamics in a wide remotely doped quantum well are studied theoretically and experimentally. Assuming that all electrons in the quantum well are localized, the theory considers the resonant interaction of light pulses with the four-level system formed by the electron spins of the ground state and the hole spins of the trion excited state. The theory describes the effects of spontaneous emission, a transverse magnetic field and hole spin relaxation on the dynamics detected by the Kerr rotation of a probe pulse. Time resolved Kerr rotation experiments were carried out on a remotely doped 14 nm GaAs quantum well in the frequency range of optical transitions to the heavy hole (HH) trion and to the light-hole (LH) trion degenerate with the HH exciton. The experiments on the resonant excitation of the HH trion show a very slow heavy hole spin relaxation and, consequently, a weak electron spin polarization after the trion relaxation. In contrast, the resonant excitation of the LH trion/HH exciton results in a fast hole spin relaxation that increases electron spin polarization.
Low frequency spin dynamics in a quantum Hall canted antiferromagnet
NASA Astrophysics Data System (ADS)
Muraki, Koji
2007-03-01
In quantum Hall (QH) systems, Coulomb interactions combined with the macroscopic degeneracy of Landau levels (LLs) drive the electron system into strongly correlated phases as illustrated by the series of fractional QH effects and may also lead to various forms of broken symmetry dictated by the LL filing factor ν. When two layers of such electron systems are closely separated by a thin tunnel barrier, the addition of interlayer interactions and the layer degree of freedom brings about even richer electronic phases, opening up possibilities for different classes of symmetry breaking. In particular, at total filling factor νT = 2, where the two of the four lowest LLs split by the Zeeman and interlayer tunnel couplings are occupied, the competing degrees of freedom due to the layer and spin are predicted to lead to rich magnetic phases. Here we present results of resistively detected nuclear spin relaxation measurements in closely separated electron systems that reveal strong low-frequency spin fluctuations in the QH regime at νT = 2 [1]. As the temperature is decreased, the spin fluctuations, manifested by a sharp enhancement of the nuclear spin-lattice relaxation rate 1/T1, continue to grow down to the lowest temperature of 66 mK. The observed divergent behavior of 1/T1 signals a gapless spin excitation mode (i.e., a Goldstone mode) and is a hallmark of the theoretically predicted canted antiferromagnetic order. Our data demonstrate the realization of a two-dimensional system with broken planar spin rotational symmetry, in which fluctuations do not freeze out when approaching the zero temperature limit. [1] N. Kumada, K. Muraki, and Y. Hirayama, Science 313, 329 (2006).
Low energy spin dynamics in the spin ice, Ho2Sn2O7
Ehlers, Georg; Huq, Ashfia; Diallo, Souleymane Omar; Adriano, Cris; Rule, K; Cornelius, A. L.; Fouquet, Peter; Pagliuso, P G; Gardner, Jason
2012-01-01
The magnetic properties of Ho{sub 2}Sn{sub 2}O{sub 7} have been investigated and compared to other spin ice compounds. Although the lattice has expanded by 3% relative to the better studied Ho{sub 2}Ti{sub 2}O{sub 7} spin ice, no significant changes were observed in the high temperature properties, T {approx}> 20 K. As the temperature is lowered and correlations develop, Ho{sub 2}Sn{sub 2}O{sub 7} enters its quantum phase at a slightly higher temperature than Ho{sub 2}Ti{sub 2}O{sub 7} and is more antiferromagnetic in character. Below 80 K a weak inelastic mode associated with the holmium nuclear spin system has been measured. The hyperfine field at the holmium nucleus was found to be {approx}700 T.
Dynamics of Polymer Blend Film Formation During Spin Coating
NASA Astrophysics Data System (ADS)
Mouhamad, Youmna; Clarke, Nigel; Jones, Richard A. L.; Geoghegan, Mark
2012-02-01
Spin casting is a process broadly used to obtain a uniform film on a flat substrate. A homogeneous film results from the balance between centrifugal and viscous forces. Here we revisit the Meyerhofer model of the spin casting process by taking in account the centrifugal forces, a uniform time dependent evaporation rate, and account for the changes in viscosity using the Huggins intrinsic viscosity. Time resolved light reflectometry is used to monitor the thickness changes of a polystyrene-poly(methyl methacrylate)(which we denote as PS and PMMA) film initially dissolved in toluene and spin cast for ten seconds at 1000 rpm. The experimental data are in good agreement with the model. We also investigate how the volume fraction of PS and PMMA influences the thinning of the film during spin casting. A distinct change in the temporal evolution of thickness as a function of time delimits the first phase of the spin casting process where centrifugal forces are dominant from a second phase dominated by the solvent evaporation. This hypothesis is supported by in-situ off specular scattering data. The time at which this change from centrifugal to evaporation-dominated behaviour is delayed as the volume fraction of PMMA increases.
Spin dynamics and Kondo physics in optical tweezers
NASA Astrophysics Data System (ADS)
Lin, Yiheng; Lester, Brian J.; Brown, Mark O.; Kaufman, Adam M.; Long, Junling; Ball, Randall J.; Isaev, Leonid; Wall, Michael L.; Rey, Ana Maria; Regal, Cindy A.
2016-05-01
We propose to use optical tweezers as a toolset for direct observation of the interplay between quantum statistics, kinetic energy and interactions, and thus implement minimum instances of the Kondo lattice model in systems with few bosonic rubidium atoms. By taking advantage of strong local exchange interactions, our ability to tune the spin-dependent potential shifts between the two wells and complete control over spin and motional degrees of freedom, we design an adiabatic tunneling scheme that efficiently creates a spin-singlet state in one well starting from two initially separated atoms (one atom per tweezer) in opposite spin state. For three atoms in a double-well, two localized in the lowest vibrational mode of each tweezer and one atom in an excited delocalized state, we plan to use similar techniques and observe resonant transfer of two-atom singlet-triplet states between the wells in the regime when the exchange coupling exceeds the mobile atom hopping. Moreover, we argue that such three-atom double-tweezers could potentially be used for quantum computation by encoding logical qubits in collective spin and motional degrees of freedom. Current address: Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA.
Optical and spin polarization dynamics in GaSe nanoslabs
NASA Astrophysics Data System (ADS)
Tang, Yanhao; Xie, Wei; Mandal, Krishna C.; McGuire, John A.; Lai, C. W.
2015-05-01
We report nearly complete preservation of "spin memory" between optical absorption and photoluminescence (PL) in nanometer slabs of GaSe pumped with up to 0.2 eV excess energy. At cryogenic temperatures, the initial degree of circular polarization (ρ0) of PL approaches unity, with the major fraction of the spin polarization decaying with a time constant >500 ps in sub-100-nm GaSe nanoslabs. Even at room temperature, ρ0 as large as 0.7 is observed, while pumping 1 eV above the band edge yields ρ0=0.15 . Angular momentum preservation for both electrons and holes is due to the separation of the nondegenerate conduction and valence bands from other bands. In contrast to valley polarization in atomically thin transition-metal dichalcogenides, here optical spin polarization is preserved in nanoslabs of 100 layers or more of GaSe.
Effect of surfactant and solvent on spin-lattice relaxation dynamics of magnetic nanocrystals.
Maiti, Sourav; Chen, Hsiang-Yun; Chen, Tai-Yen; Hsia, Chih-Hao; Son, Dong Hee
2013-04-25
The effect of varying the surfactant and solvent medium on the dynamics of spin-lattice relaxation in photoexcited Fe3O4 nanocrystals has been investigated by measuring the time-dependent magnetization employing pump-probe transient Faraday rotation technique. The variation of the surfactants having surface-binding functional groups modified not only the static magnetization but also the dynamics of the recovery of the magnetization occurring via spin-lattice relaxation in the photoexcited Fe3O4 nanocrystals. The variation of the polarity and size of the solvent molecules can also influence the spin-lattice relaxation dynamics. However, the effect is limited to the nanocrystals having sufficiently permeable surfactant layer, where the small solvent molecules (e.g., water) can access the surface and dynamically modify the ligand field on the surface. PMID:23003213
Dynamic consequences of optical spin-orbit interaction
NASA Astrophysics Data System (ADS)
Sukhov, Sergey; Kajorndejnukul, Veerachart; Naraghi, Roxana Rezvani; Dogariu, Aristide
2015-12-01
Field symmetries and conservation laws are closely associated through Noether's theorem. Light field inhomogeneities lead to changes in linear and angular momenta and, consequently, to radiation pressure, spin or rotation of objects. Here we discuss a new type of mechanical action originating in the exchange between spin and orbital angular momenta. We demonstrate theoretically and experimentally that, when mirror and central symmetries of scattering are broken, a force appears acting perpendicularly to the direction of propagation. This new force completes the set of non-conservative forces (radiation pressure and tractor beams) that can be generated with unstructured light beams.
Unraveling Photoinduced Spin Dynamics in the Topological Insulator Bi(2)Se(3).
Wang, M C; Qiao, S; Jiang, Z; Luo, S N; Qi, J
2016-01-22
We report on a time-resolved ultrafast optical spectroscopy study of the topological insulator Bi_{2}Se_{3}. We unravel that a net spin polarization cannot only be generated using circularly polarized light via interband transitions between topological surface states (SSs), but also via transitions between SSs and bulk states. Our experiment demonstrates that tuning photon energy or temperature can essentially allow for photoexcitation of spin-polarized electrons to unoccupied topological SSs with two distinct spin relaxation times (∼25 and ∼300 fs), depending on the coupling between SSs and bulk states. The intrinsic mechanism leading to such distinctive spin dynamics is the scattering in SSs and bulk states which is dominated by E_{g}^{2} and A_{1g}^{1} phonon modes, respectively. These findings are suggestive of novel ways to manipulate the photoinduced coherent spins in topological insulators. PMID:26849605
Coherent spin dynamics of donor bound electrons in GaAs
NASA Astrophysics Data System (ADS)
Phelps, Carey; O'Leary, Shannon; Prineas, John; Wang, Hailin
2011-08-01
We report experimental studies of coherent spin dynamics of donor-bound electrons in high-purity GaAs by using transient differential transmission. The donor-bound exciton transitions, which are not visible in the linear absorption spectrum, are spectrally resolved in the nonlinear differential transmission spectra. The spin beats in the transient differential transmission response, arising from electron spin precession in an external magnetic field, are investigated with the pump and probe coupling to various donor-bound exciton transitions. The spectral dependence of the spin beats provides important information on the polarization selection rule for the underlying donor-bound exciton transitions. The polarization selection rules deduced from these experiments indicate that contributions from higher-energy donor-bound exciton transitions can severely limit the effectiveness of optical spin control using mechanisms such as polarization-dependent optical Stark shifts.
Constrained spin-density dynamics of an iron-sulfur complex: Ferredoxin cofactor
NASA Astrophysics Data System (ADS)
Ali, Md. Ehesan; Nair, Nisanth N.; Staemmler, Volker; Marx, Dominik
2012-06-01
The computation of antiferromagnetic exchange coupling constants J by means of efficient density-based approaches requires in practice to take care of both spin projection to approximate the low spin ground state and proper localization of the magnetic orbitals at the transition metal centers. This is demonstrated here by a combined approach where the extended broken-symmetry (EBS) technique is employed to include the former aspect, while spin density constraints are applied to ensure the latter. This constrained EBS (CEBS) approach allows us to carry out ab initio molecular dynamics on a spin-projected low spin potential energy surface that is generated on-the-fly by propagating two coupled determinants and thereby accessing the antiferromagnetic coupling along the trajectory. When applied to the prototypical model of the oxidized [2Fe-2S] cofactor in Ferredoxins, [Fe2S2(SH)4]2-, at room temperature, CEBS leads to remarkably good results for geometrical structures and coupling constants J.
Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO_{4}
Toft-Petersen, Rasmus; Reehuis, Manfred; Jensen, Thomas B. S.; Andersen, Niels H.; Li, Jiying; Le, Manh Duc; Laver, Mark; Niedermayer, Christof; Klemke, Bastian; Lefmann, Kim; Vaknin, David
2015-07-06
We report significant details of the magnetic structure and spin dynamics of LiFePO_{4} obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis. In addition, we find a significant spin-canting component along c. Furthermore, the possible causes of these components are discussed, and their significance for the magnetoelectric effect is analyzed. Inelastic neutron scattering along the three principal directions reveals a highly anisotropic hard plane consistent with earlier susceptibility measurements. While using a spin Hamiltonian, we show that the spin dimensionality is intermediate between XY- and Ising-like, with an easy b axis and a hard c axis. As a result, it is shown that both next-nearest neighbor exchange couplings in the bc plane are in competition with the strongest nearest neighbor coupling.
NASA Astrophysics Data System (ADS)
Haag, M.; van den Brandt, B.; Eichhorn, T. R.; Hautle, P.; Wenckebach, W. Th.
2012-06-01
In a test of principle a neutron spin filter has been built, which is based on dynamic nuclear polarization (DNP) using photo-excited triplet states. This DNP method has advantages over classical concepts as the requirements for cryogenic equipment and magnets are much relaxed: the spin filter is operated in a field of 0.3 T at a temperature of about 100 K and has performed reliably over periods of several weeks. The neutron beam was also used to analyze the polarization of the target employed as a spin filter. We obtained an independent measurement of the proton spin polarization of ˜0.13 in good agreement with the value determined with NMR. Moreover, the neutron beam was used to measure the proton spin polarization as a function of position in the naphthalene sample. The polarization was found to be homogeneous, even at low laser power, in contradiction to existing models describing the photo-excitation process.
NASA Astrophysics Data System (ADS)
Kumar, Krishan; Garg, Vinayak; Moudgil, R. K.
2013-06-01
We report a theoretical study on the spin-resolved pair-correlation functions gσσ'(r) of a two-dimensional electron gas having arbitrary spin polarization ζ by including the dynamics of exchange-correlations within the dynamical self-consistent mean-field theory of Hasegawa and Shimizu. The calculated g↑↑(r), g↓↓(r) and g↑↓(r) exhibit a nice agreement with the recent quantum Monte Carlo simulation data of Gori-Giorgi et al. However, the agreement for the minority spin correlation function g↓↓(r) decreases with increase in ζ and/or decrease in electron density. Nevertheless, the spin-summed correlation function remains close to the simulation data.
Weyl fermions and spin dynamics of metallic ferromagnet SrRuO3
Itoh, Shinichi; Endoh, Yasuo; Yokoo, Tetsuya; Ibuka, Soshi; Park, Je-Geun; Kaneko, Yoshio; Takahashi, Kei S.; Tokura, Yoshinori; Nagaosa, Naoto
2016-01-01
Weyl fermions that emerge at band crossings in momentum space caused by the spin–orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet. PMID:27273207
Solid effect DNP polarization dynamics in a system of many spins
NASA Astrophysics Data System (ADS)
Wiśniewski, Daniel; Karabanov, Alexander; Lesanovsky, Igor; Köckenberger, Walter
2016-03-01
We discuss the polarization dynamics during solid effect dynamic nuclear polarization (DNP) in a central spin model that consists of an electron surrounded by many nuclei. To this end we use a recently developed formalism and validate first its performance by comparing its predictions to results obtained by solving the Liouville von Neumann master equation. The use of a Monte Carlo method in our formalism makes it possible to significantly increase the number of spins considered in the model system. We then analyse the dependence of the nuclear bulk polarization on the presence of nuclei in the vicinity of the electron and demonstrate that increasing the minimal distance between nuclei and electrons leads to a rise of the nuclear bulk polarization. These observations have implications for the design of radicals that can lead to improved values of nuclear spin polarization. Furthermore, we discuss the potential to extend our formalism to more complex spin systems such as cross effect DNP.
Neutrino spin dynamics in dense matter and electromagnetic field
NASA Astrophysics Data System (ADS)
Arbuzova, E. V.
2008-11-01
We discuss behavior of massive Dirac neutrino with anomalous magnetic moment propagating through dense magnetized matter on the basis of the obtained solutions of the Dirac-Pauli equation. This system of solutions demonstrates spin rotating properties and represents pure neutrino states.
Clustering and decoherence of correlated spins under double quantum dynamics
NASA Astrophysics Data System (ADS)
Sánchez, Claudia M.; Acosta, Rodolfo H.; Levstein, Patricia R.; Pastawski, Horacio M.; Chattah, Ana K.
2014-10-01
We present an improved approach for the study of the evolution of spin correlations and decoherence in multiple quantum nuclear magnetic resonance experiments. The infinite system, constituted by the protons of a polycrystalline adamantane sample, evolves under a double quantum Hamiltonian. The distribution of multiple quantum coherence orders is represented by a contribution of spin clusters with different sizes that exchange spins, increasing their size with the evolution time. A cluster with nearly exponential growth at all times is observed, in agreement with previous models. Remarkably, a small cluster that stabilizes in a size corresponding to 18 correlated spins is revealed. In addition, by performing a renormalization of the obtained data with the experimental Loschmidt echo, the contribution of the different clusters to the observable signal is determined. This procedure accounts for the effect of decoherence on the evolution of the system, and allows setting the range of confidence of the experimental data. Our analysis confirms the natural hint that, correlated states involving higher coherence orders are far more sensitive to the uncontrolled decoherent interactions, than those involving lower orders.
Charge dynamics and spin blockade in a hybrid double quantum dot in silicon
NASA Astrophysics Data System (ADS)
Chatterjee, Anasua; Urdampilleta, Matias; Lo, Cheuk Chi; Mansir, John; Barraud, Sylvain; Betz, Andreas; Gonzalez-Zalba, M. Fernando; Morton, John J. L.
Hybrid architectures combining donor atoms and quantum dots in silicon can take advantage of fast gate voltage based spin manipulations to form a hybrid singlet-triplet qubit, with access to the quantum memory offered by the nuclear spin of the donor via the hyperfine interaction. Additionally, spin buses using quantum dot chains could mediate the transfer of quantum information between long-lived donor spins. We present an approach to a novel hybrid double quantum dot by coupling a donor to an artificial atom in a CMOS-compatible nanotransistor. Using gate-based RF-reflectometry, we probe the charge stability of the system and its quantum capacitance. Through microwave spectroscopy, we find a tunnel coupling of 2.7GHz and characterize the charge dynamics, revealing a charge T1 of 100ns. We also show spin blockade at the inderdot transition and investigate the spin dynamics, opening up the possibility to operate this coupled system as a singlet-triplet qubit and to coherently transfer spin information between the quantum dot and the donor electron and nucleus. We acknowledge support from the TOLOP project (FP7/318397), the EPSRC, ARC, and the UNDEDD project, the Royal Commission for the Exhibition of 1851 and the Royal Society.
Impurity and boundary effects on magnetic monopole dynamics in spin ice
NASA Astrophysics Data System (ADS)
Kycia, J. B.; Revell, H. M.; Yaraskavitch, L. R.; Mason, J. D.; Ross, K. A.; Noad, H. M. L.; Dabkowska, H. A.; Gaulin, B. D.; Henelius, P.
2013-03-01
Using a SQUID magnetometer, we measure the time-dependent magnetic relaxation in Dy2Ti2O7 and find that it decays with a stretched exponential followed by a very slow long-time tail. In a Monte Carlo simulation governed by Metropolis dynamics we find that surface effects and a very low level of stuffed spins (0.30%) - magnetic Dy ions substituted for non-magnetic Ti ions - can explain these signatures in the relaxation. We find that the additional spins trap the magnetic monopole excitations and provide the first example of how defects in a spin-ice material can obstruct the flow of monopoles.
Neutron Scattering Study on spin dynamics in superconducting (TlRb)2Fe4Se5
Chi, Songxue; Ye, Feng; Bao, Wei; Fang, Dr. Minghu; Wang, H.D.; Dong, C.H.; Savici, Andrei T; Granroth, Garrett E; Stone, Matthew B; Fishman, Randy Scott
2013-01-01
Spin dynamics in superconducting (Tl,Rb)2Fe4Se5 was investigated using the inelastic neutron scattering technique. Spin wave branches that span an energy range from 6.5 to 209 meV are success- fully described by a Heisenberg model whose dominant interactions include only the in-plane nearest (J1 and J0 1) and next nearest neighbor (J2 and J0 2) exchange terms within and between the tetramer spin blocks, respectively. These exchange constants, experimentally determined in this work, would crucially constrain the diverse theoretical viewpoints on magnetism and superconductivity in the Fe-based materials.
Nonlinear magnetic vortex dynamics in a circular nanodot excited by spin-polarized current
2014-01-01
We investigate analytically and numerically nonlinear vortex spin torque oscillator dynamics in a circular magnetic nanodot induced by a spin-polarized current perpendicular to the dot plane. We use a generalized nonlinear Thiele equation including spin-torque term by Slonczewski for describing the nanosize vortex core transient and steady orbit motions and analyze nonlinear contributions to all forces in this equation. Blue shift of the nano-oscillator frequency increasing the current is explained by a combination of the exchange, magnetostatic, and Zeeman energy contributions to the frequency nonlinear coefficient. Applicability and limitations of the standard nonlinear nano-oscillator model are discussed. PMID:25147490
Finite-Temperature Entanglement Dynamics in an Anisotropic Two-Qubit Heisenberg Spin Chain
NASA Astrophysics Data System (ADS)
Chen, Tao; Shan, Chuanjia; Li, Jinxing; Liu, Tangkun; Huang, Yanxia; Li, Hong
2010-07-01
This paper investigates the entanglement dynamics of an anisotropic two-qubit Heisenberg spin chain in the presence of decoherence at finite temperature. The time evolution of the concurrence is studied for different initial Werner states. The influences of initial purity, finite temperature, spontaneous decay and Hamiltonian on the entanglement evolution are analyzed in detail. Our calculations show that the finite temperature restricts the evolution of the entanglement all the time when the Hamiltonian improves it and the spontaneous decay to the reservoirs can produce quantum entanglement with the anisotropy of spin-spin interaction. Finally, the steady-state concurrence which may remain non-zero for low temperature is also given.
Evidence of spin glass dynamics in dilute LiHoxY1-xF4.
Quilliam, J A; Meng, S; Mugford, C G A; Kycia, J B
2008-10-31
ac susceptibility measurements are presented on the dilute, dipolar coupled, Ising magnet LiHoxY1-xF4 for a concentration x=0.045. The frequency and temperature dependences of the susceptibility show characteristic glassy relaxation. The absorption spectrum is found to broaden with decreasing temperature suggesting that the material is behaving as a spin glass and not as an exotic spin liquid as was previously observed. A dynamical scaling analysis suggests a spin glass transition temperature of 43+/-2 mK with an exponent znu=7.8+/-0.2. PMID:18999860
Evidence of Spin Glass Dynamics in Dilute LiHoxY1-xF4
NASA Astrophysics Data System (ADS)
Quilliam, J. A.; Meng, S.; Mugford, C. G. A.; Kycia, J. B.
2008-10-01
ac susceptibility measurements are presented on the dilute, dipolar coupled, Ising magnet LiHoxY1-xF4 for a concentration x=0.045. The frequency and temperature dependences of the susceptibility show characteristic glassy relaxation. The absorption spectrum is found to broaden with decreasing temperature suggesting that the material is behaving as a spin glass and not as an exotic spin liquid as was previously observed. A dynamical scaling analysis suggests a spin glass transition temperature of 43±2mK with an exponent zν=7.8±0.2.
Modeling Dynamical Black Holes with Spin Parameters Larger Than 0.999
NASA Astrophysics Data System (ADS)
Ruchlin, Ian; Etienne, Zachariah
2016-03-01
Exploring the extremal Kerr limit in a dynamical, fully general relativistic context may lend insights into the no-hair theorem and uncover new mechanisms by which black hole spins can be increased beyond astrophysical or Kerr limits. Modeling such black holes is highly challenging, with state-of-the-art numerical relativity simulations reaching spin parameters of 0.99 to 0.995 only recently. We have developed new techniques that open the door to stable and reliable puncture black hole evolutions with spin parameters in excess of 0.999. We briefly review these techniques, the results, and possible applications.
Dynamics of spin valves investigated using Magneto-Optical Kerr Effect Spectroscopy
NASA Astrophysics Data System (ADS)
Stevens, Christopher; Paul, Jagannath; Dey, Prasenjit; Miller, Casey; McGill, Stephen; Karaiskaj, Denis
Through an all-optical approach, we are investigating the spin dynamics in different spin torque based structures. Using pump-probe Time-Resolved Magneto-Optical Kerr Effect (TR-MOKE) spectroscopy, we are able to monitor the ultrafast magnon propagation on a sub-picosecond timescale as well as the longer lived oscillations and demagnetization. This represents a recent efforts to realize magnon induced spin torque using an all optical method. This research at USF is supported by the National Science Foundation, Division of Electrical, Communications and Cyber Systems under Grant Number: 1231929. The work was done in part at the NHMFL, Tallahassee, FSU under Grants: DMR-1229217, DMR-1157490.
Spin-Wave Theory for the Dynamics Induced by Direct Currents in Magnetic Multilayers
NASA Astrophysics Data System (ADS)
Rezende, S. M.; de Aguiar, F. M.; Azevedo, A.
2005-01-01
A spin-wave theory is presented for the magnetization dynamics in a ferromagnetic film that is traversed by spin-polarized carriers at high direct-current densities. It is shown that nonlinear effects due to four-magnon interactions arising from dipolar and surface anisotropy energies limit the growth of the driven spin wave and produce shifts in the microwave frequency oscillations. The theory explains quantitatively recent experimental results in nanometric point contacts onto magnetic multilayers showing downward frequency shifts (redshifts) with increasing current, if the external field is on the film plane, and upward shifts (blueshifts), if the field is perpendicular to the film.
The dynamics of particle disks. II - Effects of spin degrees of freedom
NASA Technical Reports Server (NTRS)
Araki, Suguru
1988-01-01
The present treatment of the thermal equilibria of differentially-rotating, axisymmetric disks consisting of identical, spin-possessing as well as translational DOF-possessing hard sphere particles characterizes these disks' dynamics by means of two novel parameters: (1) the tangential restitution coefficient, and (2) the dimensionless moment of inertia. It is established that rings composed of spinning particles can generally be thermally balanced within more restricted ranges of the optical depth, as well as at higher values of the normal restitution coefficient, than spinless rings. Mean spin is indefinite in the present framework of neglected finite particle-size effects.
Large-amplitude spin dynamics driven by a THz pulse in resonance with an electromagnon.
Kubacka, T; Johnson, J A; Hoffmann, M C; Vicario, C; de Jong, S; Beaud, P; Grübel, S; Huang, S-W; Huber, L; Patthey, L; Chuang, Y-D; Turner, J J; Dakovski, G L; Lee, W-S; Minitti, M P; Schlotter, W; Moore, R G; Hauri, C P; Koohpayeh, S M; Scagnoli, V; Ingold, G; Johnson, S L; Staub, U
2014-03-21
Multiferroics have attracted strong interest for potential applications where electric fields control magnetic order. The ultimate speed of control via magnetoelectric coupling, however, remains largely unexplored. Here, we report an experiment in which we drove spin dynamics in multiferroic TbMnO3 with an intense few-cycle terahertz (THz) light pulse tuned to resonance with an electromagnon, an electric-dipole active spin excitation. We observed the resulting spin motion using time-resolved resonant soft x-ray diffraction. Our results show that it is possible to directly manipulate atomic-scale magnetic structures with the electric field of light on a sub-picosecond time scale. PMID:24603154
Duchstein, Patrick; Milek, Theodor; Zahn, Dirk
2015-01-01
Molecular models of 5 nm sized ZnO/Zn(OH)2 core-shell nanoparticles in ethanolic solution were derived as scale-up models (based on an earlier model created from ion-by-ion aggregation and self-organization) and subjected to mechanistic analyses of surface stabilization by block-copolymers. The latter comprise a poly-methacrylate chain accounting for strong surfactant association to the nanoparticle by hydrogen bonding and salt-bridges. While dangling poly-ethylene oxide chains provide only a limited degree of sterical hindering to nanoparticle agglomeration, the key mechanism of surface stabilization is electrostatic shielding arising from the acrylates and a halo of Na+ counter ions associated to the nanoparticle. Molecular dynamics simulations reveal different solvent shells and distance-dependent mobility of ions and solvent molecules. From this, we provide a molecular rationale of effective particle size, net charge and polarizability of the nanoparticles in solution. PMID:25962096
Lee, Jong Min; Jang, Chaun; Min, Byoung-Chul; Lee, Seo-Won; Lee, Kyung-Jin; Chang, Joonyeon
2016-01-13
Dzyaloshinskii-Moriya interaction (DMI), which arises from the broken inversion symmetry and spin-orbit coupling, is of prime interest as it leads to a stabilization of chiral magnetic order and provides an efficient manipulation of magnetic nanostructures. Here, we report all-electrical measurement of DMI using propagating spin wave spectroscopy based on the collective spin wave with a well-defined wave vector. We observe a substantial frequency shift of spin waves depending on the spin chirality in Pt/Co/MgO structures. After subtracting the contribution from other sources to the frequency shift, it is possible to quantify the DMI energy in Pt/Co/MgO systems. The result reveals that the DMI in Pt/Co/MgO originates from the interfaces, and the sign of DMI corresponds to the inversion asymmetry of the film structures. The electrical excitation and detection of spin waves and the influence of interfacial DMI on the collective spin-wave dynamics will pave the way to the emerging field of spin-wave logic devices. PMID:26653115
Molecular dynamics in paramagnetic materials as studied by magic-angle spinning 2H NMR spectra.
Mizuno, Motohiro; Suzuki, You; Endo, Kazunaka; Murakami, Miwa; Tansho, Masataka; Shimizu, Tadashi
2007-12-20
A magic-angle spinning (MAS) 2H NMR experiment was applied to study the molecular motion in paramagnetic compounds. The temperature dependences of 2H MAS NMR spectra were measured for paramagnetic [M(H2O)6][SiF6] (M=Ni2+, Mn2+, Co2+) and diamagnetic [Zn(H2O)6][SiF6]. The paramagnetic compounds exhibited an asymmetric line shape in 2H MAS NMR spectra because of the electron-nuclear dipolar coupling. The drastic changes in the shape of spinning sideband patterns and in the line width of spinning sidebands due to the 180 degrees flip of water molecules and the reorientation of [M(H2O)6]2+ about its C3 axis were observed. In the paramagnetic compounds, paramagnetic spin-spin relaxation and anisotropic g-factor result in additional linebroadening of each of the spinning sidebands. The spectral simulation of MAS 2H NMR, including the effects of paramagnetic shift and anisotropic spin-spin relaxation due to electron-nuclear dipolar coupling and anisotropic g-factor, was performed for several molecular motions. Information about molecular motions in the dynamic range of 10(2) s(-1)
Spin dynamics and relaxation in graphene nanoribbons: electron spin resonance probing.
Rao, Singamaneni S; Stesmans, Andre; van Tol, Johan; Kosynkin, Dmitry V; Higginbotham-Duque, A; Lu, Wei; Sinitskii, Alexander; Tour, James M
2012-09-25
Here we report the results of a multifrequency (~9, 20, 34, 239.2, and 336 GHz) variable-temperature continuous wave (cw) and X-band (~9 GHz) pulse electron spin resonance (ESR) measurement performed at cryogenic temperatures on potassium split graphene nanoribbons (GNRs). Important experimental findings include the following: (a) The multifrequency cw ESR data infer the presence of only carbon-related paramagnetic nonbonding states, at any measured temperature, with the g value independent of microwave frequency and temperature. (b) A linear broadening of the ESR signal as a function of microwave frequency is noticed. The observed linear frequency dependence of ESR signal width points to a distribution of g factors causing the non-Lorentzian line shape, and the g broadening contribution is found to be very small. (c) The ESR process is found to be characterized by slow and fast components, whose temperature dependences could be well described by a tunneling level state model. This work not only could help in advancing the present fundamental understanding on the edge spin (or magnetic)-based properties of GNRs but also pave the way to GNR-based spin devices. PMID:22901098
NASA Astrophysics Data System (ADS)
Teale, Andrew M.; Lutnæs, Ola B.; Helgaker, Trygve; Tozer, David J.; Gauss, Jürgen
2013-01-01
Accurate sets of benchmark nuclear-magnetic-resonance shielding constants and spin-rotation constants are calculated using coupled-cluster singles-doubles (CCSD) theory and coupled-cluster singles-doubles-perturbative-triples [CCSD(T)] theory, in a variety of basis sets consisting of (rotational) London atomic orbitals. The accuracy of the calculated coupled-cluster constants is established by a careful comparison with experimental data, taking into account zero-point vibrational corrections. Coupled-cluster basis-set convergence is analyzed and extrapolation techniques are employed to estimate basis-set-limit quantities, thereby establishing an accurate benchmark data set. Together with the set provided for rotational g-tensors and magnetizabilities in our previous work [O. B. Lutnæs, A. M. Teale, T. Helgaker, D. J. Tozer, K. Ruud, and J. Gauss, J. Chem. Phys. 131, 144104 (2009)], 10.1063/1.3242081, it provides a substantial source of consistently calculated high-accuracy data on second-order magnetic response properties. The utility of this benchmark data set is demonstrated by examining a wide variety of Kohn-Sham exchange-correlation functionals for the calculation of these properties. None of the existing approximate functionals provide an accuracy competitive with that provided by CCSD or CCSD(T) theory. The need for a careful consideration of vibrational effects is clearly illustrated. Finally, the pure coupled-cluster results are compared with the results of Kohn-Sham calculations constrained to give the same electronic density. Routes to future improvements are discussed in light of this comparison.
Slow Spin Dynamics in Superconducting Ca0.9Ce0.1Fe2As2
Nadeem, K.; Zhang, W.; Chen, D. Y.; Ren, Z. A.; Qiu, X. G.
2015-01-01
Slow spin dynamics has been observed in superconducting under-doped Ca0.9Ce0.1Fe2As2 single crystal. Below 100 K, the system exhibits hysteresis in the cooling and warming protocols of temperature dependent resistivity due to first order tetragonal to orthorhombic structural transition with simultaneous magnetic transition from paramagnetic to spin density wave antiferromagnetic state of the iron (Fe) ions. Zero field cooled/field cooled (ZFC/FC) magnetization curves showed splitting at 32 K followed by a sharp increase of the FC curve and then FC plateau at low temperatures. Slow spin relaxation in both the ZFC and FC protocols was observed which is typical for spin-glass system. The system also showed features analogue to spin-glass behavior such as ZFC peak, FC plateau, ZFC slow spin relaxation, magnetic hysteresis, and ZFC ac memory effect. The spin-glass like behavior was rather weak and vanished at higher fields. The origin of the slow spin dynamics could be the inhomogeneous distribution of the cerium (Ce) spins ordered along the c-axis OR interactions between Fe and Ce spins which lead to magnetic frustration of Ce spins. All these findings support the coexistence of slow spin dynamics of Ce spins and superconductivity in Ca0.9Ce0.1Fe2As2 single crystal. PMID:26024047
Optimal Controller Tested for a Magnetically Suspended Five-Axis Dynamic Spin Rig
NASA Technical Reports Server (NTRS)
Choi, Benjamin B.
2003-01-01
NASA Glenn Research Center's Structural Mechanics and Dynamics Branch has developed a fully suspended magnetic bearing system for their Dynamic Spin Rig, which performs vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust magnetic bearing and the associated control system were integrated into the Dynamic Spin Rig to provide magnetic excitation as well as noncontact magnetic suspension of the 35-lb vertical rotor with blades to induce turbomachinery blade vibration (ref. 1). The new system can provide longer run times at higher speeds and larger vibration amplitudes for rotating blades. Also, it was proven that bearing mechanical life was substantially extended and flexibility was increased in the excitation orientation (direction and phasing).
NASA Astrophysics Data System (ADS)
Balian, S. J.; Liu, Ren-Bao; Monteiro, T. S.
2015-06-01
There are two distinct techniques of proven effectiveness for extending the coherence lifetime of spin qubits in environments of other spins. One is dynamical decoupling, whereby the qubit is subjected to a carefully timed sequence of control pulses; the other is tuning the qubit towards "optimal working points" (OWPs), which are sweet spots for reduced decoherence in magnetic fields. By means of quantum many-body calculations, we investigate the effects of dynamical decoupling pulse sequences far from and near OWPs for a central donor qubit subject to decoherence from a nuclear spin bath. Key to understanding the behavior is to analyze the degree of suppression of the usually dominant contribution from independent pairs of flip-flopping spins within the many-body quantum bath. We find that to simulate recently measured Hahn echo decays at OWPs (lowest-order dynamical decoupling), one must consider clusters of three interacting spins since independent pairs do not even give finite-T2 decay times. We show that while operating near OWPs, dynamical decoupling sequences require hundreds of pulses for a single order of magnitude enhancement of T2, in contrast to regimes far from OWPs, where only about 10 pulses are required.
Effect of modularity on the Glauber dynamics of the dilute spin glass model
NASA Astrophysics Data System (ADS)
Park, Jeong-Man
2014-11-01
We study the Glauber dynamics of the dilute, infinite-ranged spin glass model, the so-called dilute Sherrington-Kirkpatrick (dSK) model. The dSK model has sparse couplings and can be classified by the modularity ( M) of the coupling matrix. We investigate the effect of the modularity on the relaxation dynamics starting from a random initial state. By using the Glauber dynamics and the replica method, we derive the relaxation dynamics equations for the magnetization ( m) and the energy per spin ( r), in addition to the equation for the spin glass order parameter ( q αβ ). In the replica symmetric (RS) analysis, we find that there are two solutions for the RS spin glass order parameter ( q): q = 0which is stable for r < 1/2 and q = (-1+4 r 2)/(32 r 4) which is stable for r > 1/2 in the non-modular system and q = 0 which is stable for r < 1/ and q = (-1+8 r 2)/(128 r 4) which is stable for r > 1/ in the completely modular system. By substituting the proper q values into the equations for r, we find that the relaxation dynamics of r depends on the modularity, M. These results suggest that, in the context of evolutionary theory, the modularity may emerge spontaneously in the point-mutation-only framework (Glauber dynamics) under a changing environment.
Attitude dynamic of spin-stabilized satellites with flexible appendages
NASA Technical Reports Server (NTRS)
Renard, M. L.
1973-01-01
Equations of motion and computer programs have been developed for analyzing the motion of a spin-stabilized spacecraft having long, flexible appendages. Stability charts were derived, or can be redrawn with the desired accuracy for any particular set of design parameters. Simulation graphs of variables of interest are readily obtainable on line using program FLEXAT. Finally, applications to actual satellites, such as UK-4 and IMP-1 have been considered.
Flight dynamics of a spinning projectile descending on a parachute
Benedetti, G.A.
1989-02-01
During the past twenty years Sandia National Laboratories and the US Army have vertically gun launched numerous 155mm and eight-inch diameter flight test projectiles. These projectiles are subsequently recovered using an on-board parachute recovery system which is attached to the forward case structure of the projectile. There have been at least five attempts to describe, through analytical and numerical simulations, the translational and rotational motions of a spinning projectile descending on a parachute. However, none of these investigations have correctly described the large nutational motion of the projectile since all of them overlooked the fundamental mechanism which causes these angular motions. Numerical simulations as well as a closed form analytical solution show conclusively that the Magnus moment is responsible for the large nutational motion of the projectile. That is, when the center of pressure for the Magnus force is aft of the center of mass for the projectile, the Magnus moment causes an unstable (or large) nutational motion which always tends to turn the spinning projectile upside down while it is descending on the parachute. Conversely, when the center of mass for the projectile is aft of the center of pressure for the Magnus force, the Magnus moment stabilizes the nutational motion tending to always point the base of the spinning projectile down. The results of this work are utilized to render projectile parachute recovery systems more reliable and to explain what initially may appear to be strange gyrodynamic behavior of a spinning projectile descending on a parachute. 14 refs., 20 figs.
Spin dynamics in SiGe quantum dot lines and ring molecules
NASA Astrophysics Data System (ADS)
Zinovieva, A. F.; Nenashev, A. V.; Dvurechenskii, A. V.
2016-04-01
Semiconductor quantum dot (QD) structures can be used as a model for understanding the effect of the microscopic structure, symmetry of crystals, and molecules on their macroscopic properties. In this work, the results of two theoretical approaches demonstrate that the spin dynamics in ordered QD structures depends on the size, spatial configuration, and topology of the object built of QDs. It was shown that the spin dynamics in QD structures with the hopping regime of conductivity significantly differs from the spin dynamics in two-dimensional (2D) and three-dimensional (3D) structures being at the other side of the metal-insulator transition. The special character of the effective magnetic field δ H fluctuations appearing only during tunneling between quantum dots is responsible for the insensitivity of spin relaxation times to the magnitude of the external magnetic field in infinite QD structures (2D square lattice and 1D linear QD chain). In finite QD structures (QD rings and linear chains), an external magnetic field H0 is directly involved in the spin relaxation process and spin is lost due to interaction with a special combination of fields Δ H ˜[H0×δ H ]/δ H that leads to an unusual orientation dependence of ESR linewidth, recently observed for QD chains. It was shown that the ordering of QD structures can be used for the conservation of spin orientation. For 1D finite quantum dot chains, the ordering can provide the stabilization of all spin components Sx,Sy, and Sz, while for ringlike molecules only Sz polarization can be stabilized. The results obtained in this work can be useful for development of novel semiconductor devices and in quantum information processing.
Benedetti, G.A.
1990-11-01
When a fluid flows inside a tube, the deformations of the tube can interact with the fluid flowing within it and these dynamic interactions can result in significant lateral motions of the tube and the flowing fluid. The purpose of this report is to examine the dynamic stability of a spinning tube through which an incompressible frictionless fluid is flowing. The tube can be considered as either a hollow beam or a hollow cable. The analytical results can be applied to spinning or stationary tubes through which fluids are transferred; e.g., liquid coolants, fuels and lubricants, slurry solutions, and high explosives in paste form. The coupled partial differential equations are determined for the lateral motion of a spinning Bernoulli-Euler beam or a spinning cable carrying an incompressible flowing fluid. The beam, which spins about an axis parallel to its longitudinal axis and which can also be loaded by a constant axial force, is straight, uniform, simply supported, and rests on a massless, uniform elastic foundation that spins with the beam. Damping for the beam and foundation is considered by using a combined uniform viscous damping coefficient. The fluid, in addition to being incompressible, is frictionless, has a constant density, and flows at a constant speed relative to the longitudinal beam axis. The Galerkin method is used to reduce the coupled partial differential equations for the lateral motion of the spinning beam to a coupled set of 2N, second order, ordinary differential equations for the generalized beam coordinates. By simplifying these equations and examining the roots of the characteristic equation, an analytical solution is obtained for the lateral dynamic instability of the beam (or cable). The analytical solutions determined the minimum critical fluid speed and the critical spin speeds, for a specified fluid speed, in terms of the physical parameters of the system.
NASA Astrophysics Data System (ADS)
Artemieva, Irina; Shulgin, Alexey
2015-04-01
Mesoproterozoic mafic magmatism at the southern part of the Baltic Shield (the Lake Ladoga region) is conventionally ascribed to epicratonic rifting. The region hosts a series of mafic dykes and sills of Mesoproterozoic ages, including a ca. 1.53-1.46 Ga sheet-like gabbro-dolerite sills and the Salmi plateau-basalts from the Lake Ladoga region. Based on chiefly geochemical data, the region is conventionally interpreted as an intracratonic Ladoga rift (graben). We question the validity of this geodynamic interpretation by analyzing regional geophysical data (crustal structure, heat flow, Bouguer gravity anomalies, magnetic anomalies, and mantle Vs velocities). Our analysis of characteristics of continental rifts demonstrates that: 1. the topography of the region lacks a linear horst-graben structure typical of modern rifts, however this feature might have been lost by surface erosion; 2. the crust has neither shallow Moho, nor magmatic high-velocity underplated material, and thus is not typical of continental rifts; 3. weakly negative Bouguer gravity anomalies, especially by comparison with adjacent "background" anomalies suggest the presence of high-density material at shallow, near-Moho depths; however, the shape of the anomaly is rounded rather than linear, and may not attest to the paleorifting event; 4. seismic velocities in the upper mantle show a possible weak low-Pn anomaly near Lake Ladoga, and strong positive (+5+7%) Vs anomaly at 75-125 km depth to the NE of the lake, but not in the region of Mesoproterozoic mafic magmatism; 5. no thermal anomaly or lithosphere thickness anomaly is currently present in the lithosphere of the region, which instead is marked by extremely low heat flow; however, given the age of magmatism any thermal anomaly may have long ceased and thus its absence does not disprove rifting origin of magmatism; 6. the absence of linear magnetic anomalies which are preserved in other paleorifts provides strong evidence that this region has
Non-markovian mesoscopic dissipative dynamics of open quantum spin chains
NASA Astrophysics Data System (ADS)
Benatti, F.; Carollo, F.; Floreanini, R.; Narnhofer, H.
2016-01-01
We study the dissipative dynamics of N quantum spins with Lindblad generator consisting of operators scaling as fluctuations, namely with the inverse square-root of N. In the large N limit, the microscopic dissipative time-evolution converges to a non-Markovian unitary dynamics on strictly local operators, while at the mesoscopic level of fluctuations it gives rise to a dissipative non-Markovian dynamics. The mesoscopic time-evolution is Gaussian and exhibits either a stable or an unstable asymptotic character; furthermore, the mesoscopic dynamics builds correlations among fluctuations that survive in time even when the original microscopic dynamics is unable to correlate local observables.
RosettaEPR: Rotamer Library for Spin Label Structure and Dynamics
Alexander, Nathan S.; Stein, Richard A.; Koteiche, Hanane A.; Kaufmann, Kristian W.; Mchaourab, Hassane S.; Meiler, Jens
2013-01-01
An increasingly used parameter in structural biology is the measurement of distances between spin labels bound to a protein. One limitation to these measurements is the unknown position of the spin label relative to the protein backbone. To overcome this drawback, we introduce a rotamer library of the methanethiosulfonate spin label (MTSSL) into the protein modeling program Rosetta. Spin label rotamers were derived from conformations observed in crystal structures of spin labeled T4 lysozyme and previously published molecular dynamics simulations. Rosetta’s ability to accurately recover spin label conformations and EPR measured distance distributions was evaluated against 19 experimentally determined MTSSL labeled structures of T4 lysozyme and the membrane protein LeuT and 73 distance distributions from T4 lysozyme and the membrane protein MsbA. For a site in the core of T4 lysozyme, the correct spin label conformation (Χ1 and Χ2) is recovered in 99.8% of trials. In surface positions 53% of the trajectories agree with crystallized conformations in Χ1 and Χ2. This level of recovery is on par with Rosetta performance for the 20 natural amino acids. In addition, Rosetta predicts the distance between two spin labels with a mean error of 4.4 Å. The width of the experimental distance distribution, which reflects the flexibility of the two spin labels, is predicted with a mean error of 1.3 Å. RosettaEPR makes full-atom spin label modeling available to a wide scientific community in conjunction with the powerful suite of modeling methods within Rosetta. PMID:24039810
Bhattacharjee, Satadeep; Nordström, Lars; Fransson, Jonas
2012-02-01
We consider spin dynamics for implementation in an atomistic framework and we address the feasibility of capturing processes in the femtosecond regime by inclusion of moment of inertia. In the spirit of an s-d-like interaction between the magnetization and electron spin, we derive a generalized equation of motion for the magnetization dynamics in the semiclassical limit, which is nonlocal in both space and time. Using this result we retain a generalized Landau-Lifshitz-Gilbert equation, also including the moment of inertia, and demonstrate how the exchange interaction, damping, and moment of inertia, all can be calculated from first principles. PMID:22400957
Density Functional Plus Dynamical Mean Field Study of Spin Crossover Molecule
NASA Astrophysics Data System (ADS)
Chen, Jia; Millis, Andrew; Marianetti, Chris
2015-03-01
We report a density functional plus dynamical mean field study of spin crossover molecule Fe(phen)2(NCS)2. The temperature dependent magnetic susceptibility, Fe-d spectral and total energy were calculated and compared with experimental magnetization, metal L-edge x-ray adsorption spectroscopy. The importance of dynamic effect on energetics is demonstrated by comparison with density functional plus U method, and the role of full charge self-consistency is identified. Moreover, the local spin density plus U (LSDA+U) method with exchange interaction explicitly included is shown to dramatically overemphasize magnetic interaction.
Lattice Dynamics of EuO: Evidence for Giant Spin-Phonon Coupling.
Pradip, R; Piekarz, P; Bosak, A; Merkel, D G; Waller, O; Seiler, A; Chumakov, A I; Rüffer, R; Oleś, A M; Parlinski, K; Krisch, M; Baumbach, T; Stankov, S
2016-05-01
Comprehensive studies of lattice dynamics in the ferromagnetic semiconductor EuO have been performed by a combination of inelastic x-ray scattering, nuclear inelastic scattering, and ab initio calculations. A remarkably large broadening of the transverse acoustic phonons was discovered at temperatures above and below the Curie temperature T_{C}=69 K. This result indicates a surprisingly strong momentum-dependent spin-phonon coupling induced by the spin dynamics in EuO. PMID:27203332
Tuning the spin dynamics of single molecule magnets via dipolar interactions
NASA Astrophysics Data System (ADS)
Hofmann, A.; Salman, Z.
2014-12-01
We present calculations of the dipolar field distribution acting on a single molecule magnet due to its neighbours in thin films. The calculations are presented for different packing/configuration scenarios, with different easy axis orientations. The potential for controlling the molecular spin dynamics by tuning the molecule-substrate interaction and its competition with intra-molecular interactions is discussed. We argue that by altering the configuration of the molecular moments, and thus their dipolar interactions, one can enhance or slow down their spin dynamics.
Effect of thermal fluctuations in spin-torque driven magnetization dynamics
NASA Astrophysics Data System (ADS)
Bonin, R.; Bertotti, G.; Serpico, C.; Mayergoyz, I. D.; d'Aquino, M.
2007-09-01
Nanomagnets with uniaxial symmetry driven by an external field and spin-polarized currents are considered. Anisotropy, applied field, and spin polarization are all aligned along the symmetry axis. Thermal fluctuations are described by adding a Gaussian white noise stochastic term to the Landau-Lifshitz-Gilbert equation for the deterministic dynamics. The corresponding Fokker-Planck equation is derived. It is shown that deterministic dynamics, thermal relaxation, and transition rate between stable states are governed by an effective potential including the effect of current injection.
Geometric phases and quantum correlations dynamics in spin-boson model
Wu, Wei; Xu, Jing-Bo
2014-01-28
We explore the dynamics of spin-boson model for the Ohmic bath by employing the master equation approach and obtain an explicit expression of reduced density matrix. We also calculate the geometric phases of the spin-boson model by making use of the analytical results and discuss how the dissipative bosonic environment affects geometric phases. Furthermore, we investigate the dynamics of quantum discord and entanglement of two qubits each locally interacting with its own independent bosonic environments. It is found that the decay properties of quantum discord and entanglement are sensitive to the choice of initial state's parameter and coupling strength between system and bath.
NASA Astrophysics Data System (ADS)
Komatsu, Keiji; Ono, Syuji; Shimizu, Junichiro; Nagashima, Ryuichi
Two experiments are carried out to investigate the dynamic behavior of the liquid partially filled in spherical tanks of a spinning satellite. One is the simulation test at the spin up phase of the rocket. The other is the sloshing test to analyze the propellant sloshing effects on the satellite attitude control. These experiments are specially set for the Engineering Test Satellite V which has two spherical tanks 37 percent filled with hydrazine, but the results obtained can be applicable to the other problems of the liquid dynamics in spherical tanks.
A spin-wave logic gate based on a width-modulated dynamic magnonic crystal
Nikitin, Andrey A.; Ustinov, Alexey B.; Semenov, Alexander A.; Kalinikos, Boris A.; Chumak, Andrii V.; Serga, Alexander A.; Vasyuchka, Vitaliy I.; Hillebrands, Burkard; Lähderanta, Erkki
2015-03-09
An electric current controlled spin-wave logic gate based on a width-modulated dynamic magnonic crystal is realized. The device utilizes a spin-wave waveguide fabricated from a single-crystal Yttrium Iron Garnet film and two conducting wires attached to the film surface. Application of electric currents to the wires provides a means for dynamic control of the effective geometry of waveguide and results in a suppression of the magnonic band gap. The performance of the magnonic crystal as an AND logic gate is demonstrated.
Soh, Wee Tee Ong, C. K.; Peng, Bin
2015-08-15
The spin rectification effect (SRE), a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR) as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG) spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs) of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO{sub 2} spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.
NASA Astrophysics Data System (ADS)
Soh, Wee Tee; Peng, Bin; Ong, C. K.
2015-08-01
The spin rectification effect (SRE), a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR) as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG) spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs) of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO2 spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.
Nonlinear Dynamics of Magnons observed by AC Spin Pumping in Magnetic Hybrid Structures
NASA Astrophysics Data System (ADS)
Vilela-Leao, L. H.; Cunha, R. O.; Azevedo, A.; Rodriguez-Suarez, R. L.; Rezende, S. M.
2015-03-01
The electron spin degree of freedom constitutes the basic means to carry and store information in the field of spintronics. In the spin pumping process, the microwave driven magnetization dynamics in a ferromagnetic film generates a spin current in an attached metallic layer that can be converted into a charge current by means of the inverse spin Hall effect and detected by a voltage signal. While the time independent component (DC) of the spin current has been widely investigated in a variety of material structures, recently it has been recognized that the alternating current (AC) component is much larger, though more difficult to detect, and has many attractive features. We report experiments with microwave driven DC and AC spin pumping in bilayers made of the insulating ferrimagnet yttrium iron garnet (YIG) and platinum that reveal the nonlinear dynamics involving the driven mode and a pair of magnon modes with half frequency. This process occurs when the frequency is lowered below a critical value so that a three-magnon splitting process with energy conservation is made possible. The results are explained by a model with coupled nonlinear equations describing the time evolution of the magnon modes.
Dynamics and control of flexible spinning solar sails under reflectivity modulation
NASA Astrophysics Data System (ADS)
Mu, Junshan; Gong, Shengping; Ma, Pengbin; Li, Junfeng
2015-10-01
Electrochromic devices have been used for the attitude control of a spinning solar sail in a deep space mission by modulating the reflectivity of the sail membrane. As a flexible spinning solar sail has no rigid structure to support its membrane, the distributed load due to solar radiation will lead to the deformation of the sail membrane, and the control torque generated by reflectivity modulation can introduce oscillatory motion to the membrane. By contrast, the deformation and oscillatory motion of the sail membrane have an impact on the performance of the reflectivity control. This paper investigates the dynamics and control of flexible spinning solar sails under reflectivity modulation. The static deformation of a spinning sail membrane subjected to solar radiation pressure in an equilibrium state is analyzed. The von Karman theory is used to obtain the displacements and the stress distribution in the equilibrium states. A simplified analytical first-order mode is chosen to model the membrane oscillation. The coupled membrane oscillation-attitude-orbit dynamics are considered for a GeoSail formation flying mission. The relative attitude and orbit control of flexible spinning solar sails under reflectivity modulation are numerically tested. The simulations indicate that the membrane deformation and oscillation have a lower impact on the control of the reflectivity modulated sails than the increase of the spinning rate.
Hovav, Yonatan; Feintuch, Akiva; Vega, Shimon
2013-01-01
Dynamic nuclear polarization is a method which allows for a dramatic increase of the NMR signals due to polarization transfer between electrons and their neighboring nuclei, via microwave irradiation. These experiments have become popular in recent years due to the ability to create hyper-polarized chemically and biologically relevant molecules, in frozen glass forming mixtures containing free radicals. Three mechanisms have been proposed for the polarization transfer between electrons and their surrounding nuclei in such non-conducting samples: the solid effect and cross effect mechanisms, which are based on quantum mechanics and relaxation on small spin systems, and thermal mixing, which originates from the thermodynamic macroscopic notion of spin temperature. We have recently introduced a spin model, which is based on the density matrix formalism and includes relaxation, and applied it to study the solid effect and cross effect mechanisms on small spin systems. In this publication we use the same model to describe the thermal mixing mechanism, and the creation of spin temperature. This is obtained without relying on the spin temperature formalism. Simulations of small model systems are used on systems with homogeneously and inhomogeneously broadened EPR lines. For the case of a homogeneously broadened line we show that the nuclear enhancement results from the thermal mixing and solid effect mechanisms, and that spin temperatures are created in the system. In the inhomogeneous case the enhancements are attributed to the solid effect and cross effect mechanisms, but not thermal mixing. PMID:23160533
Hyperfine and spin-orbit dynamics in GaAs double quantum dots
NASA Astrophysics Data System (ADS)
Shulman, Michael; Nichol, John; Harvey, Shannon; Pal, Arijeet; Halperin, Bertrand; Umansky, Vladimir; Yacoby, Amir
2015-03-01
Semiconductor quantum dots provide a unique platform for single-particle physics and many-body quantum mechanics. In particular, understanding the dynamics of a single electron interacting with a nuclear spin bath is key to improving spin-based quantum information processing, since the hyperfine interaction limits the performance of many spin qubits. We probe the electron-nuclear interaction by measuring the splitting at the anti-crossing between the electron singlet (S) and m =1 triplet (T +) states in a GaAs double quantum dot. Using Landau-Zener sweeps, we find that the size of this splitting varies by more than an order of magnitude depending on the magnitude and direction of the external magnetic field. These results are consistent with a competition between the spin orbit interaction and the hyperfine interaction, even though the extracted spin orbit length is much larger than the size of the double quantum dot. We confirm these results by using Landau-Zener sweeps to measure the high-frequency correlations in the S-T + splitting that arise from the Larmor precession of the nuclei. These unexpected results have implications for improving the performance of spin-based quantum information processing, as well as improving our understanding of the central spin problem.
Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes
NASA Astrophysics Data System (ADS)
Mi, Bin-Zhou
2016-09-01
The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green's function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.
Chaotic dynamics of stellar spin in binaries and the production of misaligned hot Jupiters.
Storch, Natalia I; Anderson, Kassandra R; Lai, Dong
2014-09-12
Many exoplanetary systems containing hot Jupiters are observed to have highly misaligned orbital axes relative to the stellar spin axes. Kozai-Lidov oscillations of orbital eccentricity and inclination induced by a binary companion, in conjunction with tidal dissipation, constitute a major channel for the production of hot Jupiters. We demonstrate that gravitational interaction between the planet and its oblate host star can lead to chaotic evolution of the stellar spin axis during Kozai cycles. As parameters such as the planet mass and stellar rotation period are varied, periodic islands can appear in an ocean of chaos, in a manner reminiscent of other dynamical systems. In the presence of tidal dissipation, the complex spin evolution can leave an imprint on the final spin-orbit misalignment angles. PMID:25214623
Low field domain wall dynamics in artificial spin-ice basis structure
NASA Astrophysics Data System (ADS)
Kwon, J.; Goolaup, S.; Lim, G. J.; Kerk, I. S.; Chang, C. H.; Roy, K.; Lew, W. S.
2015-10-01
Artificial magnetic spin-ice nanostructures provide an ideal platform for the observation of magnetic monopoles. The formation of a magnetic monopole is governed by the motion of a magnetic charge carrier via the propagation of domain walls (DWs) in a lattice. To date, most experiments have been on the static visualization of DW propagation in the lattice. In this paper, we report on the low field dynamics of DW in a unit spin-ice structure measured by magnetoresistance changes. Our results show that reversible DW propagation can be initiated within the spin-ice basis. The initial magnetization configuration of the unit structure strongly influences the direction of DW motion in the branches. Single or multiple domain wall nucleation can be induced in the respective branches of the unit spin ice by the direction of the applied field.
Mance, Deni; Baldus, Marc; Gast, Peter; Huber, Martina; Ivanov, Konstantin L.
2015-06-21
We develop a theoretical description of Dynamic Nuclear Polarization (DNP) in solids under Magic Angle Spinning (MAS) to describe the magnetic field dependence of the DNP effect. The treatment is based on an efficient scheme for numerical solution of the Liouville-von Neumann equation, which explicitly takes into account the variation of magnetic interactions during the sample spinning. The dependence of the cross-effect MAS-DNP on various parameters, such as the hyperfine interaction, electron-electron dipolar interaction, microwave field strength, and electron spin relaxation rates, is analyzed. Electron spin relaxation rates are determined by electron paramagnetic resonance measurements, and calculations are compared to experimental data. Our results suggest that the observed nuclear magnetic resonance signal enhancements provided by MAS-DNP can be explained by discriminating between “bulk” and “core” nuclei and by taking into account the slow DNP build-up rate for the bulk nuclei.
Dynamic properties of magnets with spin S = 3/2 and non-Heisenberg isotropic interaction
Kosmachev, O. A.; Fridman, Yu. A.; Galkina, E. G.; Ivanov, B. A.
2015-02-15
The dynamic properties of a magnet with magnetic-ion spin of 3/2 and an isotropic spin interaction of a general form have been investigated. Only four phase states can be realized in the system under consideration at various relationships between the material parameters: the ferro- and antiferromagnetic phases with saturated spin and the states with tensor order parameters, the nematic and antinematic ones. For these phases, the spontaneous symmetry breaking is determined by the octupole order parameter containing the mean values trilinear in spin operator components at a given site. The spectra of elementary excitations have been determined in all phases. Additional branches of excitations arise in all four phase states.
NASA Astrophysics Data System (ADS)
Mance, Deni; Gast, Peter; Huber, Martina; Baldus, Marc; Ivanov, Konstantin L.
2015-06-01
We develop a theoretical description of Dynamic Nuclear Polarization (DNP) in solids under Magic Angle Spinning (MAS) to describe the magnetic field dependence of the DNP effect. The treatment is based on an efficient scheme for numerical solution of the Liouville-von Neumann equation, which explicitly takes into account the variation of magnetic interactions during the sample spinning. The dependence of the cross-effect MAS-DNP on various parameters, such as the hyperfine interaction, electron-electron dipolar interaction, microwave field strength, and electron spin relaxation rates, is analyzed. Electron spin relaxation rates are determined by electron paramagnetic resonance measurements, and calculations are compared to experimental data. Our results suggest that the observed nuclear magnetic resonance signal enhancements provided by MAS-DNP can be explained by discriminating between "bulk" and "core" nuclei and by taking into account the slow DNP build-up rate for the bulk nuclei.
Low field domain wall dynamics in artificial spin-ice basis structure
Kwon, J.; Goolaup, S.; Lim, G. J.; Kerk, I. S.; Lew, W. S.; Chang, C. H.; Roy, K.
2015-10-28
Artificial magnetic spin-ice nanostructures provide an ideal platform for the observation of magnetic monopoles. The formation of a magnetic monopole is governed by the motion of a magnetic charge carrier via the propagation of domain walls (DWs) in a lattice. To date, most experiments have been on the static visualization of DW propagation in the lattice. In this paper, we report on the low field dynamics of DW in a unit spin-ice structure measured by magnetoresistance changes. Our results show that reversible DW propagation can be initiated within the spin-ice basis. The initial magnetization configuration of the unit structure strongly influences the direction of DW motion in the branches. Single or multiple domain wall nucleation can be induced in the respective branches of the unit spin ice by the direction of the applied field.
Spin crossover in ferropericlase from first-principles molecular dynamics simulations
NASA Astrophysics Data System (ADS)
Holmstrom, Eero; Stixrude, Lars
2014-05-01
Ferropericlase is the second-most abundant mineral of the lower mantle of the Earth. It is experimentally known that with increasing pressure, the iron ions in the mineral begin to collapse from a high-spin to low-spin state. This spin crossover alters various properties of the material, and hence a good theoretical understanding of the phenomenon is necessary. Using first-principles molecular dynamics simulations in conjunction with thermodynamic integration, we construct a phase diagram of the spin crossover as a function of pressure and temperature. In addition, we present the thermal equation of state of the mineral up to 140 GPa and 4000 K, and predict that the electrical conductivity of ferropericlase reaches semi-metallic values within the lower mantle.
Bethe lattice approach and relaxation dynamics study of spin-crossover materials
NASA Astrophysics Data System (ADS)
Oke, Toussaint Djidjoho; Hontinfinde, Félix; Boukheddaden, Kamel
2015-07-01
Dynamical properties of Prussian blue analogs and spin-crossover materials are investigated in the framework of a Blume-Emery-Griffiths (BEG) spin-1 model, where states ±1 and 0 represent the high-spin (HS) state and the low-spin state, respectively. The quadrupolar interaction depends on the temperature in the form . Magnetic interactions are controlled by a factor such that for (), magnetic ordering is not expected. The model is exactly solved using the Bethe lattice approach for the equilibrium properties. The results are closer to those calculated by numerical simulations with suitable Arrhenius-type transition rates. The study of relaxation processes of non-equilibrium HS states revealed one-step nonlinear sigmoidal relaxation curves of the HS fraction at low temperatures. We found that increasing the magnetic interactions leads to the appearance of a plateau in the thermal hysteresis as well as in the relaxation curves of the HS fraction at low temperature.
Dynamics of a spinning spacecraft during extension of flexible appendages
NASA Astrophysics Data System (ADS)
Turner, J.; Keat, J.; Messac, A.
1984-05-01
This paper addresses the problem of analyzing the deployment of flexible appendages from a central rigid hub of a spinning spacecraft. The rigorous mathematical modeling of mass flow and changing structural configuration of the spacecraft during deployment, while the vehicle experiences small elastic deflection and small angular rate, is presented. The equations of motion are obtained in terms of integro-partial differential equations. An approximate solution for the equations of motion is obtained by using a Raleigh-Ritz method and numerical results are presented for several deployment strategies. For every instantaneous physical configuration of the spacecraft, that extension rate which will lead to unstable behavior is also determined.
Non-Markovian dynamics in chiral quantum networks with spins and photons
NASA Astrophysics Data System (ADS)
Ramos, Tomás; Vermersch, Benoît; Hauke, Philipp; Pichler, Hannes; Zoller, Peter
2016-06-01
We study the dynamics of chiral quantum networks consisting of nodes coupled by unidirectional or asymmetric bidirectional quantum channels. In contrast to familiar photonic networks where driven two-level atoms exchange photons via 1D photonic nanostructures, we propose and study a setup where interactions between the atoms are mediated by spin excitations (magnons) in 1D X X spin chains representing spin waveguides. While Markovian quantum network theory eliminates quantum channels as structureless reservoirs in a Born-Markov approximation to obtain a master equation for the nodes, we are interested in non-Markovian dynamics. This arises from the nonlinear character of the dispersion with band-edge effects, and from finite spin propagation velocities leading to time delays in interactions. To account for the non-Markovian dynamics we treat the quantum degrees of freedom of the nodes and connecting channel as a composite spin system with the surrounding of the quantum network as a Markovian bath, allowing for an efficient solution with time-dependent density matrix renormalization-group techniques. We illustrate our approach showing non-Markovian effects in the driven-dissipative formation of quantum dimers, and we present examples for quantum information protocols involving quantum state transfer with engineered elements as basic building blocks of quantum spintronic circuits.
Dynamics of a two-level system coupled to a bath of spins
NASA Astrophysics Data System (ADS)
Wang, Haobin; Shao, Jiushu
2012-12-01
The dynamics of a two-level system coupled to a spin bath is investigated via the numerically exact multilayer multiconfiguration time-dependent Hartree (ML-MCTDH) theory. Consistent with the previous work on linear response approximation [N. Makri, J. Phys. Chem. B 103, 2823 (1999)], 10.1021/jp9847540, it is demonstrated numerically that this spin-spin-bath model can be mapped onto the well-known spin-boson model if the system-bath coupling strength obeys an appropriate scaling behavior. This linear response mapping, however, may require many bath spin degrees of freedom to represent the practical continuum limit. To clarify the discrepancies resulted from different approximate treatments of this model, the population dynamics of the central two-level system has been investigated near the transition boundary between the coherent and incoherent motions via the ML-MCTDH method. It is found that increasing temperature favors quantum coherence in the nonadiabatic limit of this model, which corroborates the prediction in the previous work [J. Shao and P. Hanggi, Phys. Rev. Lett. 81, 5710 (1998)], 10.1103/PhysRevLett.81.5710 based on the non-interacting blip approximation (NIBA). However, the coherent-incoherent boundary obtained by the exact ML-MCTDH simulation is slightly different from the approximate NIBA results. Quantum dynamics in other physical regimes are also discussed.
Magnetization dynamics under heat current in metallic spin valves and in insulators
NASA Astrophysics Data System (ADS)
Yu, Haiming
Spin caloritronics, an emerging branch of spintronics, studying the addition of thermal effects to the electrical and magnetic properties of nanostructures, has recently seen a rapid development. It has been predicted by Hatami et al. that a heat current can exert a spin torque on the magnetization in a nanostructure, analogous to the well-known spin-transfer torque induced by an electrical current. We provided the experimental evidence for the thermal spin-transfer torque effect in spin valves, showing the switching field change with heat current. I will present measurements of the second harmonic voltage response of Co-Cu-Co pseudo-spinvalves deposited in the middle of Cu nanowires. Both the magnitude of the second harmonic response of the spin valve and the field value of the maximum response are found to be dependent on the heat current. Both effects show that the magnetization dynamics of the pseudo-spinvalves is influenced by the heat current. Thus, the data provide a quantitative estimate of the thermal spin torque exerted on the magnetization of the Co layers. In addition, I will present recent study on the magnetization dynamics in a magnetic insulator YIG film under in-plane heat current. The ferromagnetic resonance linewidth is found to be tuned by the applied temperature gradient, i.e. narrowing and broadening. This suggests that the Gilbert damping parameter is compensated or reinforced by the applied temperature gradient in respective direction. These observations can be understood as a heat-driven spin torque in magnetic insulators.
Dynamics of polymer film formation during spin coating
NASA Astrophysics Data System (ADS)
Mouhamad, Y.; Mokarian-Tabari, P.; Clarke, N.; Jones, R. A. L.; Geoghegan, M.
2014-09-01
Standard models explaining the spin coating of polymer solutions generally fail to describe the early stages of film formation, when hydrodynamic forces control the solution behavior. Using in situ light scattering alongside theoretical and semi-empirical models, it is shown that inertial forces (which initially cause a vertical gradient in the radial solvent velocity within the film) play a significant role in the rate of thinning of the solution. The development of thickness as a function of time of a solute-free liquid (toluene) and a blend of polystyrene and poly(methyl methacrylate) cast from toluene were fitted to different models as a function of toluene partial pressure. In the case of the formation of the polymer blend film, a concentration-dependent (Huggins) viscosity formula was used to account for changes in viscosity during spin coating. A semi-empirical model is introduced, which permits calculation of the solvent evaporation rate and the temporal evolution of the solute volume fraction and solution viscosity.
Dynamics of polymer film formation during spin coating
Mouhamad, Y.; Clarke, N.; Jones, R. A. L.; Geoghegan, M.; Mokarian-Tabari, P.
2014-09-28
Standard models explaining the spin coating of polymer solutions generally fail to describe the early stages of film formation, when hydrodynamic forces control the solution behavior. Using in situ light scattering alongside theoretical and semi-empirical models, it is shown that inertial forces (which initially cause a vertical gradient in the radial solvent velocity within the film) play a significant role in the rate of thinning of the solution. The development of thickness as a function of time of a solute-free liquid (toluene) and a blend of polystyrene and poly(methyl methacrylate) cast from toluene were fitted to different models as a function of toluene partial pressure. In the case of the formation of the polymer blend film, a concentration-dependent (Huggins) viscosity formula was used to account for changes in viscosity during spin coating. A semi-empirical model is introduced, which permits calculation of the solvent evaporation rate and the temporal evolution of the solute volume fraction and solution viscosity.
Hole Surface Trapping Dynamics Directly Monitored by Electron Spin Manipulation in CdS Nanocrystals.
Li, Xiao; Feng, Donghai; Tong, Haifang; Jia, Tianqing; Deng, Li; Sun, Zhenrong; Xu, Zhizhan
2014-12-18
A new detection technique, pump-spin orientation-probe ultrafast spectroscopy, is developed to study the hole trapping dynamics in colloidal CdS nanocrystals. The hole surface trapping process spatially separates the electron-hole pairs excited by the pump pulse, leaves the core negatively charged, and thus enhances the electron spin signal generated by the orientation pulse. The spin enhancement transients as a function of the pump-orientation delay reveal a fast and a slow hole trapping process with respective time constants of sub-10 ps and sub-100 ps, orders of magnitude faster than that of carrier recombination. The power dependence of hole trapping dynamics elucidates the saturation process and relative number of traps, and suggests that there are three subpopulations of nanoparticles related to hole surface trapping, one with the fast trapping pathway only, another with the slow trapping pathway only, and the third with both pathways together. PMID:26273979
Gate control of low-temperature spin dynamics in two-dimensional hole systems
NASA Astrophysics Data System (ADS)
Kugler, M.; Andlauer, T.; Korn, T.; Wagner, A.; Fehringer, S.; Schulz, R.; Kubová, M.; Gerl, C.; Schuh, D.; Wegscheider, W.; Vogl, P.; Schüller, C.
2009-07-01
We have investigated spin and carrier dynamics of resident holes in high-mobility two-dimensional hole systems in GaAs/Al0.3Ga0.7As single-quantum wells at temperatures down to 400 mK. Time-resolved Faraday and Kerr rotation as well as time-resolved photoluminescence spectroscopy are utilized in our study. We observe long-lived hole-spin dynamics that are strongly temperature dependent, indicating that in-plane localization is crucial for hole-spin coherence. By applying a gate voltage, we are able to tune the observed hole g factor by more than 50%. Calculations of the hole g tensor as a function of the applied bias show excellent agreement with our experimental findings.
Large-amplitude spin dynamics driven by a THz pulse in resonance with an electromagnon
NASA Astrophysics Data System (ADS)
Johnson, Steven
With femtosecond time resolution, x-ray diffraction offers unique capabilities to observe directly the dynamics of long range order. When the x-ray energy is tuned near a core-level transition is is possible in many systems to selectively study the dynamics of long-range order of valence properties such as orbital ordering or magnetic spin. Here I discuss show how resonantly enhanced magnetic scattering can be used to quantitatively measure the character and magnitude of spin motion in a coherent electromagnon in TbMnO3 driven by a THz frequency electromagnetic field. We observe a 4° rotation of the antiferromagnetically ordered spin spiral plane, a result consistent with a previously published model that suggests this may be a viable route for ultrafast domain switching in multiferroics.
Exact quantum dynamics of spin systems using the positive-P representation
NASA Astrophysics Data System (ADS)
Ng, Ray; Sorensen, Erik
2011-03-01
We discuss a scheme for simulating the exact real time quantum dynamics of interacting quantum spin systems within the positive-P formalism. As model systems we study the transverse field Ising model as well as the Heisenberg model undergoing a quench away from the classical ferromagnetic ordered state. In using the positive-P representation (PPR), the dynamics of the interacting quantum spin system is mapped onto a set of stochastic differential equations (SDEs). The number of which scales linearly with the number of spins, N, compared to an exact solution through diagonalization that in the case of the Heisenberg model would require matrices exponentially large in N. This mapping is exact and can in principle be extended to higher dimensional interacting systems as well as to systems with an explicit coupling to the environment. We compare the results from using a PPR approach based on both the optical coherent states as well as SU(2) Radcliff coherent states.
A Model of Charge-Transfer Excitons: Diffusion, Spin Dynamics, and Magnetic Field Effects.
Lee, Chee Kong; Shi, Liang; Willard, Adam P
2016-06-16
In this Letter, we explore how the microscopic dynamics of charge-transfer (CT) excitons are influenced by the presence of an external magnetic field in disordered molecular semiconductors. This influence is driven by the dynamic interplay between the spin and spatial degrees of freedom of the electron-hole pair. To account for this interplay, we have developed a numerical framework that combines a traditional model of quantum spin dynamics with a stochastic coarse-grained model of charge transport. This combination provides a general and efficient methodology for simulating the effects of magnetic field on CT state dynamics, therefore providing a basis for revealing the microscopic origin of experimentally observed magnetic field effects. We demonstrate that simulations carried out on our model are capable of reproducing experimental results as well as generating theoretical predictions related to the efficiency of organic electronic materials. PMID:27237448
NASA Astrophysics Data System (ADS)
Pu, Zhengguo; Zhang, Jun; Yi, Su; Wang, Dajun; Zhang, Wenxian
2016-05-01
We theoretically investigate four types of dynamical instability, in particular the periodic and oscillatory type IO, in an antiferromagnetic spin-1 Bose-Einstein condensate in a nonzero magnetic field, by employing the coupled-mode theory and numerical method. This is in sharp contrast to the dynamical stability of the same system in zero field. Remarkably, a pattern transition from a periodic dynamical instability IO to a uniform one IIIO occurs at a critical magnetic field. All four types of dynamical instability and the pattern transition are ready to be detected in 23Na condensates within the availability of the current experimental techniques.
Dynamical symmetries and crossovers in a three-spin system with collective dissipation
NASA Astrophysics Data System (ADS)
Pigeon, S.; Xuereb, A.; Lesanovsky, I.; Garrahan, J. P.; De Chiara, G.; Paternostro, M.
2015-01-01
We consider the non-equilibrium dynamics of a simple system consisting of interacting spin-1/2 particles subjected to a collective damping. The model is close to situations that can be engineered in hybrid electro/opto-mechanical settings. Making use of large-deviation theory, we find a Gallavotti-Cohen symmetry in the dynamics of the system as well as evidence for the coexistence of two dynamical phases with different activity levels. We show that additional damping processes smooth out this behavior. Our analytical results are backed up by Monte Carlo simulations that reveal the nature of the trajectories contributing to the different dynamical phases.
Three-dimensional Computational Fluid Dynamics Investigation of a Spinning Helicopter Slung Load
NASA Technical Reports Server (NTRS)
Theorn, J. N.; Duque, E. P. N.; Cicolani, L.; Halsey, R.
2005-01-01
After performing steady-state Computational Fluid Dynamics (CFD) calculations using OVERFLOW to validate the CFD method against static wind-tunnel data of a box-shaped cargo container, the same setup was used to investigate unsteady flow with a moving body. Results were compared to flight test data previously collected in which the container is spinning.
Exploring Quantum Many-Body Spin Dynamics with Truncated Wigner Methods
NASA Astrophysics Data System (ADS)
Schachenmayer, Johannes
Recent experiments in atomic, molecular, and optical physics offer controlled and clean environments to experimentally study non-equilibrium dynamics of large many-body quantum spin-models with variable range interactions. Thus, efficient computation of such dynamics is of great importance. While in one dimension, time-dependent density matrix renormalization group methods (t-DMRG) have proven effective under certain conditions, computing dynamics in higher dimensional systems remains an outstanding challenge. Recently we formulated the discrete truncated Wigner approximation (DTWA), a semiclassical method based on the truncated Wigner approximation (TWA) that has been proven to be surprisingly accurate in predicting quench dynamics in high-dimensional lattices with up to tens of thousands of quantum spins. Here, we introduce the DTWA and show how it can compute time-evolution of quantum states in experiments that engineer spin-models with polar molecules in optical lattices or with ions in two-dimensional Penning traps. We show, how the DTWA can provide results for the time-evolution of classical and quantum correlations in quench experiments in regimes where other numerical methods are generally unreliable. We report on progress of how to incorporate higher order corrections to the method, and how to adapt it to systems with both spin and bosonic degrees of freedom.
Effects of ruthenium seed layer on the microstructure and spin dynamics of thin permalloy films
Jin Lichuan; Zhang Huaiwu; Tang Xiaoli; Bai Feiming; Zhong Zhiyong
2013-02-07
The spin dynamics and microstructure properties of a sputtered 12 nm Ni{sub 81}Fe{sub 19} thin film have been enhanced by the use of a ruthenium seed layer. Both the ferromagnetic resonance field and linewidth are enhanced dramatically as the thickness of ruthenium seed layer is increased. The surface anisotropy energy constant can also be largely tailored from 0.06 to 0.96 erg/cm{sup -2} by changing the seed layer thickness. The changes to the dynamics magnetization properties are caused by both ruthenium seed layer induced changes in the Ni{sub 81}Fe{sub 19} structure properties and surface topography properties. Roughness induced inhomogeneous linewidth broadening is also seen. The damping constant is highly tunable via the ruthenium thickness. This approach can be used to tailor both the structure and spin dynamic properties of thin Ni{sub 81}Fe{sub 19} films over a wide range. And it may benefit the applications of spin dynamics and spin current based devices.
Energy dynamics in the Heisenberg-Kitaev spin chain
NASA Astrophysics Data System (ADS)
Steinigeweg, Robin; Brenig, Wolfram
2016-06-01
We study the Heisenberg-Kitaev spin chain in order to uncover the interplay between two qualitatively different integrable points in the physics of heat transport in one dimension. Focusing on high temperatures and using analytical as well as numerical approaches within linear response theory, we explore several directions in parameter space including exchange-coupling ratios, anisotropies, and external magnetic fields. We show the emergence of purely ballistic energy transport at all integrable points, manifest in pronounced Drude weights and low-frequency suppression of regular-conductivity contributions. Moreover, off integrability, we find extended quantum chaotic regions with vanishing Drude weights and well-defined dc conductivities. In the vicinity of the Kitaev point, we observe clear signatures of the topological gap in the response function. This gap coexists with a nonzero Drude weight in the Kitaev chain.
NASA Astrophysics Data System (ADS)
Abolfath, Ramin M.; Trojnar, Anna; Roostaei, Bahman; Brabec, Thomas; Hawrylak, Pawel
2013-06-01
Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins. The exciton is described in terms of electron and heavy-hole spins interacting via exchange interaction with magnetic impurity, via hyperfine interaction with a finite number of nuclear spins and via dipole interaction with photons. The time evolution of the exciton, magnetic impurity and nuclear spins is calculated exactly between quantum jumps corresponding to exciton radiative recombination. The collapse of the wavefunction and the refilling of the quantum dot with a new spin-polarized exciton is shown to lead to the build up of magnetization of the magnetic impurity as well as nuclear spin polarization. The competition between electron spin transfer to magnetic impurity and to nuclear spins simultaneous with the creation of dark excitons is elucidated. The technique presented here opens up the possibility of studying optically induced dynamical magnetic and nuclear polarization in complex spin systems.
Zhang, Hou-Dao; Xu, Rui-Xue; Zheng, Xiao; Yan, YiJing
2015-01-14
We consider the hybrid system-bath dynamics, based on the Yan's dissipaton formalism [Y. J. Yan, J. Chem. Phys. 140, 054105 (2014)]. This theory provides a unified quasi-particle treatment on three distinct classes of quantum bath, coupled nonperturbatively to arbitrary quantum systems. In this work, to study the entangled system and bath polarization and nonlinear Fano interference, we incorporate further the time-dependent light field, which interacts with both the molecular system and the collective bath dipoles directly. Numerical demonstrations are carried out on a two-level system, with comparison between phonon and exciton baths, in both linear and nonlinear Fano interference regimes. PMID:25591343
Dynamic strain-mediated coupling of a single diamond spin to a mechanical resonator
Ovartchaiyapong, Preeti; Lee, Kenneth W.; Myers, Bryan A.; Jayich, Ania C. Bleszynski
2014-01-01
The development of hybrid quantum systems is central to the advancement of emerging quantum technologies, including quantum information science and quantum-assisted sensing. The recent demonstration of high-quality single-crystal diamond resonators has led to significant interest in a hybrid system consisting of nitrogen–vacancy centre spins that interact with the resonant phonon modes of a macroscopic mechanical resonator through crystal strain. However, the nitrogen–vacancy spin–strain interaction has not been well characterized. Here, we demonstrate dynamic, strain-mediated coupling of the mechanical motion of a diamond cantilever to the spin of an embedded nitrogen–vacancy centre. Via quantum control of the spin, we quantitatively characterize the axial and transverse strain sensitivities of the nitrogen–vacancy ground-state spin. The nitrogen–vacancy centre is an atomic scale sensor and we demonstrate spin-based strain imaging with a strain sensitivity of 3 × 10−6 strain Hz−1/2. Finally, we show how this spin-resonator system could enable coherent spin–phonon interactions in the quantum regime. PMID:25034828
Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond
Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.
2015-08-24
In this study, we demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T_{1} effects and DD microwave pulses are used to increase the transverse coherence time T_{2} from ~0.7ms up to ~30ms. Furthermore, we extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We also identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.
Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond
Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.
2015-08-24
In this study, we demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ~0.7ms up to ~30ms. Furthermore, we extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We also identify that the optimal controlmore » scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.« less
Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond
NASA Astrophysics Data System (ADS)
Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.
2015-08-01
We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ˜0.7 ms up to ˜30 ms . We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.
Charged carrier spin dynamics in ZnO quantum wells and epilayers
NASA Astrophysics Data System (ADS)
Kim, Jungtaek; Puls, J.; Sadofev, S.; Henneberger, F.
2016-01-01
Longitudinal charged carrier spin dynamics is studied for ZnO quantum wells and epilayers using the optical transition of the negatively charged exciton X- and the neutral donor bound exciton D0X , respectively. The hole spin relaxation is derived from the optical orientation of X- and D0X photoluminescence, whereas the spin relaxation of the resident electrons and donor electrons is accessed via the bleaching of the spin selective excitation process. Hole spin relaxation times of τ1s ,h of 80 and 140 ps are found for D0X and X-, respectively, which are practically independent of a magnetic field B∥ applied along the ZnO c ⃗ axis. Much longer longitudinal electron spin relaxation times in the 1 μ s range are uncovered if the hyperfine interaction is suppressed by a proper B∥. A field strength of ≈2 mT is large enough proving the extremely small value of the Overhauser field in ZnO. This is related to the very restricted number of magnetic nuclei interacting with the electron inside the volume of the exciton complex.
Advances and applications of dynamic-angle spinning nuclear magnetic resonance
Baltisberger, J.H.
1993-06-01
This dissertation describes nuclear magnetic resonance experiments and theory which have been developed to study quadrupolar nuclei (those nuclei with spin greater than one-half) in the solid state. Primarily, the technique of dynamic-angle spinning (DAS) is extensively reviewed and expanded upon in this thesis. Specifically, the improvement in both the resolution (two-dimensional pure-absorptive phase methods and DAS angle choice) and sensitivity (pulse-sequence development), along with effective spinning speed enhancement (again through choice of DAS conditions or alternative multiple pulse schemes) of dynamic-angle spinning experiment was realized with both theory and experimental examples. The application of DAS to new types of nuclei (specifically the {sup 87}Rb and {sup 85}Rb nuclear spins) and materials (specifically amorphous solids) has also greatly expanded the possibilities of the use of DAS to study a larger range of materials. This dissertation is meant to demonstrate both recent advances and applications of the DAS technique, and by no means represents a comprehensive study of any particular chemical problem.
Resolving the role of femtosecond heated electrons in ultrafast spin dynamics
Mendil, J.; Nieves, P.; Chubykalo-Fesenko, O.; Walowski, J.; Santos, T.; Pisana, S.; Münzenberg, M.
2014-01-01
Magnetization manipulation is essential for basic research and applications. A fundamental question is, how fast can the magnetization be reversed in nanoscale magnetic storage media. When subject to an ultrafast laser pulse, the speed of the magnetization dynamics depends on the nature of the energy transfer pathway. The order of the spin system can be effectively influenced through spin-flip processes mediated by hot electrons. It has been predicted that as electrons drive spins into the regime close to almost total demagnetization, characterized by a loss of ferromagnetic correlations near criticality, a second slower demagnetization process takes place after the initial fast drop of magnetization. By studying FePt, we unravel the fundamental role of the electronic structure. As the ferromagnet Fe becomes more noble in the FePt compound, the electronic structure is changed and the density of states around the Fermi level is reduced, thereby driving the spin correlations into the limit of critical fluctuations. We demonstrate the impact of the electrons and the ferromagnetic interactions, which allows a general insight into the mechanisms of spin dynamics when the ferromagnetic state is highly excited, and identifies possible recording speed limits in heat-assisted magnetization reversal. PMID:24496221
Zamponi, M; Wischnewski, A; Monkenbusch, M; Willner, L; Richter, D; Falus, P; Farago, B; Guenza, M G
2008-12-18
We present a comparison between theoretical predictions of the generalized Langevin equation for cooperative dynamics (CDGLE) and neutron spin echo data of dynamic structure factors for polyethylene melts. Experiments cover an extended range of length and time scales, providing a compelling test for the theoretical approach. Samples investigated include chains with increasing molecular weights undergoing dynamics across the unentangled to entangled transition. Measured center-of-mass (com) mean-square displacements display a crossover from subdiffusive to diffusive dynamics. The generalized Langevin equation for cooperative dynamics relates this anomalous diffusion to the presence of the interpolymer potential, which correlates the dynamics of a group of slowly diffusing molecules in a dynamically heterogeneous liquid. Theoretical predictions of the subdiffusive behavior, of its crossover to free diffusion, and of the number of macromolecules undergoing cooperative motion are in quantitative agreement with experiments. PMID:19072142
Lloveras, V; Badetti, E; Veciana, J; Vidal-Gancedo, J
2016-03-01
In this paper we report the study of the dynamics of a thermally modulated intramolecular spin exchange interaction of a novel diradical nitronyl nitroxide-substituted disulfide in solution and when it is grafted on a gold surface. The structure of this diradical was designed to have flexible chains leading to intramolecular collisions and hence spin exchange interaction, and with an appropriate binding group to be grafted on the gold surface to study its behavior on the surface. In solution, this diradical shows a strong spin exchange interaction between both radicals which is modulated by temperature, but also gold nanoparticles (AuNPs) functionalized with this diradical permit investigation of such a phenomenon in surface-grafted radicals. The spin-labelled AuNP synthesis was optimized to obtain high coverage of spin labels to lead to high spin exchange interaction. The obtained AuNPs were studied by Electron Paramagnetic Resonance (EPR), UV-Vis, and IR spectroscopies, HR-TEM microscopy, Cyclic Voltammetry (CV), Energy Dispersive X-ray analysis (EDX) and Thermogravimetric Analysis (TGA). This inorganic-organic hybrid material also showed dipolar interactions between its radicals which were confirmed by the appearance in the EPR spectra of an |Δms| = 2 transition at half-field. This signal gives direct evidence of the presence of a high-spin state and permitted us to study the nature of the magnetic coupling between the spins which was found to be antiferromagnetic. Self-Assembled Monolayers (SAMs) of these radicals on the Au (111) substrate were also prepared and studied by contact angle, X-Ray Photoelectron Spectroscopy (XPS), Time-of-Flight Secondary Ion Mass Spectrometry (ToF-SIMS), Cyclic Voltammetry and EPR. The magnetic as well as the electrochemical properties of the hybrid surfaces were studied and compared with the properties of this diradical in solution. Analogies between the properties of AuNPs with high coverage of radicals and those of SAM were
Spin dynamics in magnetic thin films and eletromagnetic properties of metamaterials
NASA Astrophysics Data System (ADS)
Cao, Rong
In this work, I have investigated the high frequency magnetic properties of a variety of novel materials by using the microwave techniques. The work consists of two parts: (1) spin dynamics study in magnetic multilayer thin films, (2) fabrication and characterization of novel magnetic materials. In the first part, we have observed nonlinear behaviors of the normal Gilbert damping G0 and the effective spin-mixing conductance g↑↓ in Pt/NiFe/Pt thin films when the incident microwave power is above a critical ac field hrf of 1.6 Oe. Both G0 and g↑↓ are affected by the coupling between spin coherent precession and spin wave modes. Our work is the first experimental demonstration of nonlinear behavior of the effective spin-mixing conductance g↑↓ . It suggests the nonlinear spin wave modes excited at high incident microwave power is detrimental to the spin pumping effect and should be avoided in future spin battery design. We have also studied the magnetization dynamic in IrMn/FeCo/Cu/NiFe/Cu spin valve through the Gilbert damping. Our results show that the Gilbert damping constant of NiFe is enhanced in antiparallel configuration when the magnetizations of both FM layers are precessing. This enhancement is induced by the dynamic exchange between the magnetizations of NiFe and FeCo layers. We have observed the dc voltage generation across the tunneling barrier while the spin precession is excited in the ferromagnetic free layer by the microwave field. The magnitude of the dc voltage peak is around few muVs with AlOx tunneling barrier. Our results directly indicate that spin current can be pumped through the tunneling barrier thus generates the dc voltage across the barrier. The results raise an important question about the role of the F/I barrier interface in spin pumping mechanism. More detailed experiment and theory studies are certainly needed, especially in MgO barrier based MTJ that could become a good candidate for realizing spin battery device. In the
Dynamical properties of three terminal magnetic tunnel junctions: Spintronics meets spin-orbitronics
Tomasello, R.; Carpentieri, M.; Finocchio, G.
2013-12-16
This Letter introduces a micromagnetic model able to characterize the magnetization dynamics in three terminal magnetic tunnel junctions, where the effects of spin-transfer torque and spin-orbit torque are taken into account. Our results predict that the possibility to separate electrically those two torque sources is very promising from a technological point of view for both next generation of nanoscale spintronic oscillators and microwave detectors. A scalable synchronization scheme based on the parallel connection of those three terminal devices is also proposed.
Wylie, Benjamin J; Dzikovski, Boris G; Pawsey, Shane; Caporini, Marc; Rosay, Melanie; Freed, Jack H; McDermott, Ann E
2015-04-01
We demonstrate that dynamic nuclear polarization of membrane proteins in lipid bilayers may be achieved using a novel polarizing agent: pairs of spin labels covalently bound to a protein of interest interacting at an intermolecular interaction surface. For gramicidin A, nitroxide tags attached to the N-terminal intermolecular interface region become proximal only when bimolecular channels forms in the membrane. We obtained signal enhancements of sixfold for the dimeric protein. The enhancement effect was comparable to that of a doubly tagged sample of gramicidin C, with intramolecular spin pairs. This approach could be a powerful and selective means for signal enhancement in membrane proteins, and for recognizing intermolecular interfaces. PMID:25828256
Reprint of : Transient dynamics of spin-polarized injection in helical Luttinger liquids
NASA Astrophysics Data System (ADS)
Calzona, A.; Carrega, M.; Dolcetto, G.; Sassetti, M.
2016-08-01
We analyze the time evolution of spin-polarized electron wave packets injected into the edge states of a two-dimensional topological insulator. In the presence of electron interactions, the system is described as a helical Luttinger liquid and injected electrons fractionalize. However, because of the presence of metallic detectors, no evidences of fractionalization are encoded in dc measurements, and in this regime the system does not show deviations from its non-interacting behavior. Nevertheless, we show that the helical Luttinger liquid nature emerges in the transient dynamics, where signatures of charge/spin fractionalization can be clearly identified.
Momentum and spin dynamics of Dirac particles at effective dimensional reduction
NASA Astrophysics Data System (ADS)
Silenko, Alexander J.; Teryaev, Oleg V.
2012-11-01
We consider the dynamics of Dirac particles moving in the curved spaces of variable dimension interpolating smoothly between 3- and 2-dimensional spaces and considered as a toy model for 2-dimensional structures in solid state physics. Performing the Foldy-Wouthuysen (FW) transformation of Dirac equation and passing to the classical limit, we derive the equations of motion of momentum and spin. The spin precesses with the variable angular velocity and may "flick" appearing in the remnant 2-dimensional space twice during the period.
Collective atomic motion and spin dynamics in a driven optical cavity
NASA Astrophysics Data System (ADS)
Stamper-Kurn, Dan
2016-05-01
Cavity quantum electrodynamics generally highlights the interchange of quantum noise and information between light and matter. I will discuss experiments in which the collective motion and spin of a trapped gas of ultracold atoms interact with and are detected by light in a single mode of a high-finesse optical cavity. I will present recent results on quantum-limited force detection, on the damping and amplification of Larmor precession through dynamical backaction, and on cavity-induced coupling between mechanical oscillators and between spin and motional degrees of freedom.
Spin pumping in the nonlinear dynamic regime of a Pt/Y3Fe5O12 heterostructure
NASA Astrophysics Data System (ADS)
Zhou, Hengan; Fan, Xiaolong; Ma, Li; Cui, Lei; Jia, Chenlong; Zhou, Shiming; Gui, Y. S.; Hu, C.-M.; Xue, Desheng
2016-05-01
Spin pumping occurred under nonlinear spin dynamic has been studied in Pt(17 nm)/Y3Fe5O12(YIG 66 nm) heterostructure. By using high power excitation, the precession angle (θc) of YIG can reach a value as high as 22°, and distinct nonlinear dynamic effects such as foldover ferromagnetic resonance spectra and nonlinear damping have been witnessed. The linear relation between the dc component of spin current and sin 2 θ c has been tested from linear to nonlinear spin dynamics regimes. Our main finding is that spin mixing conductance is a robust parameter that is independent on the amplitude and damping of the dynamic system, at least in our experiment conditions.
Coupled intertwiner dynamics: A toy model for coupling matter to spin foam models
NASA Astrophysics Data System (ADS)
Steinhaus, Sebastian
2015-09-01
The universal coupling of matter and gravity is one of the most important features of general relativity. In quantum gravity, in particular spin foams, matter couplings have been defined in the past, yet the mutual dynamics, in particular if matter and gravity are strongly coupled, are hardly explored, which is related to the definition of both matter and gravitational degrees of freedom on the discretization. However, extracting these mutual dynamics is crucial in testing the viability of the spin foam approach and also establishing connections to other discrete approaches such as lattice gauge theories. Therefore, we introduce a simple two-dimensional toy model for Yang-Mills coupled to spin foams, namely an Ising model coupled to so-called intertwiner models defined for SU (2 )k. The two systems are coupled by choosing the Ising coupling constant to depend on spin labels of the background, as these are interpreted as the edge lengths of the discretization. We coarse grain this toy model via tensor network renormalization and uncover an interesting dynamics: the Ising phase transition temperature turns out to be sensitive to the background configurations and conversely, the Ising model can induce phase transitions in the background. Moreover, we observe a strong coupling of both systems if close to both phase transitions.
NASA Astrophysics Data System (ADS)
Wang, L. L.; Lu, F. G.; Wang, H. P.; Murphy, A. B.; Tang, X. H.
2014-11-01
In gas metal arc welding, gases of different compositions are used to produce an arc plasma, which heats and melts the workpiece. They also protect the workpiece from the influence of the air during the welding process. This paper models gas metal arc welding (GMAW) processes using an in-house simulation code. It investigates the effects of the gas composition on the temperature distribution in the arc and on the molten pool dynamics in gas metal arc welding of steels. Pure argon, pure CO2 and different mixtures of argon and CO2 are considered in the study. The model is validated by comparing the calculated weld profiles with physical weld measurements. The numerical calculations reveal that gas composition greatly affects the arc temperature profile, heat transfer to the workpiece, and consequently the weld dimension. As the CO2 content in the shielding gas increases, a more constricted arc plasma with higher energy density is generated as a result of the increased current density in the arc centre and increased Lorentz force. The calculation also shows that the heat transferred from the arc to the workpiece increases with increasing CO2 content, resulting in a wider and deeper weld pool and decreased reinforcement height.
Deployment dynamics of a simplified spinning IKAROS solar sail via absolute coordinate based method
NASA Astrophysics Data System (ADS)
Zhao, Jiang; Tian, Qiang; Hu, Hai-Yan
2013-02-01
The spinning solar sail of large scale has been well developed in recent years. Such a solar sail can be considered as a rigid-flexible multibody system mainly composed of a spinning central rigid hub, a number of flexible thin tethers, sail membranes, and tip masses. A simplified interplanetary kite-craft accelerated by radiation of the Sun (IKAROS) model is established in this study by using the absolute-coordinate-based (ACB) method that combines the natural coordinate formulation (NCF) describing the central rigid hub and the absolute nodal coordinate formulation (ANCF) describing flexible parts. The initial configuration of the system in the second-stage deployment is determined through both dynamic and static analyses. The huge set of stiff equations of system dynamics is solved by using the generalized-alpha method, and thus the deployment dynamics of the system can be well understood.
Dynamics During Thrust Maneuvers of Flexible Spinning Satellites with Axial and Radial Booms
NASA Technical Reports Server (NTRS)
Longman, R. W.; Fedor, J. V.
1986-01-01
The dynamic response to operational maneuvers of spinning symmetric spacecraft with radial and axial booms was analyzed as part of the prelaunch dynamic analysis of the ISEE-3 spacecraft placed in a halo orbit around an Earth-Sun libration point, and later renamed ICE when it was directed to fly-by comet Giacobini-Zinner. The results presented use simple spacecraft models, and frequently give predictions that are good and easily obtained when the results from using a general purpose multibody dynamics program were very time consuming to obtain. Deployment of radial booms, spin-up after partial deployment, stationkeeping, and trajectory changes are analyzed. The latter two can involve both axial thrusting and pulsed radial thrusting once per revolution.
Environmentally induced quantum dynamical phase transition in the spin swapping operation
NASA Astrophysics Data System (ADS)
Álvarez, Gonzalo A.; Danieli, Ernesto P.; Levstein, Patricia R.; Pastawski, Horacio M.
2006-05-01
Quantum information processing relies on coherent quantum dynamics for a precise control of its basic operations. A swapping gate in a two-spin system exchanges the degenerate states ∣↑, ↓⟩ and ∣↓, ↑⟩. In NMR, this is achieved turning on and off the spin-spin interaction b =ΔE that splits the energy levels and induces an oscillation with a natural frequency ΔE /ℏ. Interaction of strength ℏ /τSE, with an environment of neighboring spins, degrades this oscillation within a decoherence time scale τϕ. While the experimental frequency ω and decoherence time τϕ were expected to be roughly proportional to b /ℏ and τSE, respectively, we present here experiments that show drastic deviations in both ω and τϕ. By solving the many spin dynamics, we prove that the swapping regime is restricted to ΔEτSE≳ℏ. Beyond a critical interaction with the environment the swapping freezes and the decoherence rate drops as 1/τϕ∝(b /ℏ)2τSE. The transition between quantum dynamical phases occurs when ω ∝√(b/ℏ)2-(k/τSE)2 becomes imaginary, resembling an overdamped classical oscillator. Here, 0⩽k2⩽1 depends only on the anisotropy of the system-environment interaction, being 0 for isotropic and 1 for XY interactions. This critical onset of a phase dominated by the quantum Zeno effect opens up new opportunities for controlling quantum dynamics.
Dynamical Jahn-Teller effect in spin-orbital coupled system
NASA Astrophysics Data System (ADS)
Nasu, Joji; Ishihara, Sumio
2012-02-01
Orbital degree of freedom is one of the most attractive themes in strongly correlated electron system. A coupling between the orbital and the lattice vibration is known as a Jahn-Teller effect (JTE). The dynamical aspect of the Jahn-Teller interaction is often neglected in solid, because it is strongly suppressed by the cooperative JTE. Recently, Ba3CuSb2O9 has been reported as a candidate of the spin liquid. A Cu^2+ has the eg orbital degree of freedom and is surrounded by the O^2- octahedron. The octahedra on the neighboring sites do not have the common O ions. This fact implies that the cooperative JTE is weak, and the dynamical JTE is expected to play some key roles on orbital and magnetic properties. The purpose of this research is to study the dynamical JTE in a spin-orbital coupled system. In particular, we focus on the competitive or cooperative phenomena between the superexchange interaction and the dynamical JTE. The superexchange interactions are derived from the d-p model on a honeycomb lattice. We have confirmed this interaction stabilizes the antiferro-spin and ferro-orbital configurations for the realistic parameters. The dynamical JTE described as the orbital-lattice coupling is obtained by extracting the low energy states of the vibronic Hamiltonian. We analyze the model including the two kinds of interactions by using the Bethe approximation. We find that the magnetic order is unstable in wide parameter region and the spin-dimer state with the orbital order is realized. Furthermore the orbital order is strongly suppressed by the dynamical JTE.
Dynamical effects of spin-dependent interactions in low- and intermediate-energy heavy-ion reactions
NASA Astrophysics Data System (ADS)
Xu, Jun; Li, Bao-An; Shen, Wen-Qing; Xia, Yin
2015-10-01
It is well known that noncentral nuclear forces, such as the spin-orbital coupling and the tensor force, play important roles in understanding many interesting features of nuclear structures. However, their dynamical effects in nuclear reactions are poorly known because only the spin-averaged observables are normally studied both experimentally and theoretically. Realizing that spin-sensitive observables in nuclear reactions may convey useful information about the in-medium properties of noncentral nuclear interactions, besides earlier studies using the time-dependent Hartree-Fock approach to understand the effects of spin-orbital coupling on the threshold energy and spin polarization in fusion reactions, some efforts have been made recently to explore the dynamical effects of noncentral nuclear forces in intermediate-energy heavy-ion collisions using transport models. The focus of these studies has been on investigating signatures of the density and isospin dependence of the form factor in the spin-dependent single-nucleon potential. Interestingly, some useful probes were identified in the model studies but so far there are still no data to compare with. In this brief review, we summarize the main physics motivations as well as the recent progress in understanding the spin dynamics and identifying spin-sensitive observables in heavy-ion reactions at intermediate energies. We hope the interesting, important, and new physics potentials identified in the spin dynamics of heavy-ion collisions will stimulate more experimental work in this direction.
Role of environmental correlations in the non-Markovian dynamics of a spin system
Lorenzo, Salvatore; Plastina, Francesco; Paternostro, Mauro
2011-09-15
We study the dynamics of a chain of interacting quantum particles affected by an individual or collective environment(s), focusing on the role played by the environmental quantum correlations over the evolution of the chain. The presence of entanglement in the state of the environment magnifies the non-Markovian nature of the chain's dynamics, giving rise to structures in figures of merit such as spin entanglement and purity that are not observed under a separable environmental state. Our analysis can be relevant to problems tackling the open-system dynamics of biological complexes of strong current interest.
Dynamics of entanglement in a two-dimensional spin system
Xu Qing; Sadiek, Gehad; Kais, Sabre
2011-06-15
We consider the time evolution of entanglement in a finite two-dimensional transverse Ising model. The model consists of a set of seven localized spin-(1/2) particles in a two-dimensional triangular lattice coupled through nearest-neighbor exchange interaction in the presence of an external time-dependent magnetic field. The magnetic field is applied in different function forms: step, exponential, hyperbolic, and periodic. We found that the time evolution of the entanglement shows an ergodic behavior under the effect of the time-dependent magnetic fields. Also, we found that while the step magnetic field causes great disturbance to the system, creating rapid oscillations, the system shows great controllability under the effects of the other magnetic fields where the entanglement profile follows closely the shape of the applied field even with the same frequency for periodic fields. This follow-up trend breaks down as the strength of the field, the transition constant for the exponential and hyperbolic forms, or the frequency for periodic field increase leading to rapid oscillations. We observed that the entanglement is very sensitive to the initial value of the applied periodic field: the smaller the initial value is, the less distorted the entanglement profile is. Furthermore, the effect of thermal fluctuations is very devastating to the entanglement, which decays very rapidly as the temperature increases. Interestingly, although a large value of the magnetic field strength may yield a small entanglement, the magnetic field strength was found to be more persistent against thermal fluctuations than the small field strengths.
Quantum spin dynamics and entanglement generation with hundreds of trapped ions
NASA Astrophysics Data System (ADS)
Bohnet, Justin G.; Sawyer, Brian C.; Britton, Joseph W.; Wall, Michael L.; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J.
2016-06-01
Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of 9Be+ ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods.
Finite temperature dynamics of spin-1/2 chains with symmetry breaking interactions
NASA Astrophysics Data System (ADS)
Manmana, Salvatore R.; Tiegel, Alexander C.; Pruschke, Thomas; Honecker, Andreas
I will discuss recent developments for flexible matrix product state (MPS) approaches to calculate finite-temperature spectral functions of low-dimensional strongly correlated quantum systems. The main focus will be on a Liouvillian formulation. The resulting algorithm does not specifically depend on the MPS formulation, but is applicable for any wave function based approach which can provide a purification of the density matrix, opening the way for further developments of numerical methods. Based on MPS results for various spin chains, in particular systems with Dzyaloshinskii-Moriya interactions caused by spin-orbit coupling and dimerized chains, I will discuss how symmetry breaking interactions change the nature of the finite-temperature dynamic spin structure factor obtained in ESR and neutron scattering experiments. We acknowledge funding by the Helmholtz Virtual Institute ``New States of Matter and Their Excitations''.
Quantum spin dynamics and entanglement generation with hundreds of trapped ions.
Bohnet, Justin G; Sawyer, Brian C; Britton, Joseph W; Wall, Michael L; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J
2016-06-10
Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of (9)Be(+) ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods. PMID:27284189
Snyder, Keith W.
2002-01-01
A modular system for containing projectiles has a sheet of material including at least a polycarbonate layer held by a metal frame having a straight frame member corresponding to each straight edge of the sheet. Each frame member has a U-shaped shield channel covering and holding a straight edge of the sheet and an adjacent U-shaped clamp channel rigidly held against the shield channel. A flexible gasket separates each sheet edge from its respective shield channel; and each frame member is fastened to each adjacent frame member only by clamps extending between adjacent clamp channels.
NASA Astrophysics Data System (ADS)
Maisuradze, A.; Dalmas de Réotier, P.; Yaouanc, A.; Forget, A.; Baines, C.; King, P. J. C.
2015-09-01
We report a positive muon spin relaxation and rotation (μ SR ) study of the quantum spin ice materials Yb2Ti2O7 and Yb2Sn2O7 focusing on the low field response. In agreement with earlier reports, data recorded in small longitudinal fields evidence anomalously slow spin dynamics in the microsecond range below the temperature Tc at which the specific heat displays an intense peak, namely Tc=0.24 K and 0.15 K, respectively, for the two systems. We found that slow dynamics extends above Tc up to at least 0.7 K for both compounds. The conventional dynamical Gaussian Kubo-Toyabe model describes the μ SR spectra recorded above Tc. At lower temperatures a published analytical extension of the Gaussian Kubo-Toyabe model provides a good description, consistent with the existence of short-range magnetic correlations. While the physical response of the two systems is qualitatively the same, Yb2Ti2O7 exhibits a much larger local magnetic susceptibility than Yb2Sn2O7 below Tc. Considering previously reported ac susceptibility, neutron scattering, and μ SR results, we suggest the existence of anomalously slow spin dynamics to be a common physical property of pyrochlore magnetic materials. The possibility of molecular spin substructures to be associated to the slow dynamics and therefore the short-range correlations is mentioned. The slow spin dynamics observed under field does not exclude the presence of much faster dynamics detected in extremely low or zero field.
NASA Astrophysics Data System (ADS)
Nikolić, Branislav K.; Dragomirova, Ralitsa L.
2009-06-01
We review recent studies of the shot noise of spin-polarized charge currents and pure spin currents in multiterminal semiconductor nanostructures, while focusing on the effects brought by the intrinsic Rashba spin-orbit (SO) coupling and/or extrinsic SO scattering off impurities in two-dimensional electron gas (2DEG) based devices. By generalizing the scattering theory of quantum shot noise to include the full spin-density matrix of electrons injected from a spin-filtering electrode, we show how decoherence and dephasing in the course of spin precession can lead to the substantial enhancement of the Fano factor (noise-to-current ratio) of spin-polarized charge currents. These processes are suppressed by decreasing the width of the diffusive Rashba wire, so that purely electrical measurement of the shot noise in a ferromagnet|SO-coupled-diffusive-wire|paramagnet setup can quantify the degree of quantum coherence of transported spin through a remarkable one-to-one correspondence between the purity of the spin state and the Fano factor. In four-terminal SO-coupled nanostructures, injection of unpolarized charge current through the longitudinal leads is responsible not only for the pure spin Hall current in the transverse leads, but also for nonequilibrium random time-dependent current fluctuations. The analysis of the shot noise of transverse pure spin Hall current and zero charge current, or transverse spin current and non-zero charge Hall current, driven by unpolarized or spin-polarized injected longitudinal charge current, respectively, reveals a unique experimental tool to differentiate between the intrinsic Rashba and extrinsic SO mechanisms underlying the spin Hall effect in 2DEG devices. When the intrinsic mechanisms responsible for spin precession start to dominate the spin Hall effect, they also enhance the shot noise of transverse spin and charge transport in multiterminal geometries. Finally, we discuss the shot noise of transverse spin and zero charge
Valero, Rosendo; Truhlar, Donald G
2007-09-01
A diabatic representation is convenient in the study of electronically nonadiabatic chemical reactions because the diabatic energies and couplings are smooth functions of the nuclear coordinates and the couplings are scalar quantities. A method called the fourfold way was devised in our group to generate diabatic representations for spin-free electronic states. One drawback of diabatic states computed from the spin-free Hamiltonian, called a valence diabatic representation, for systems in which spin-orbit coupling cannot be ignored is that the couplings between the states are not zero in asymptotic regions, leading to difficulties in the calculation of reaction probabilities and other properties by semiclassical dynamics methods. Here we report an extension of the fourfold way to construct diabatic representations suitable for spin-coupled systems. In this article we formulate the method for the case of even-electron systems that yield pairs of fragments with doublet spin multiplicity. For this type of system, we introduce the further simplification of calculating the triplet diabatic energies in terms of the singlet diabatic energies via Slater's rules and assuming constant ratios of Coulomb to exchange integrals. Furthermore, the valence diabatic couplings in the triplet manifold are taken equal to the singlet ones. An important feature of the method is the introduction of scaling functions, as they allow one to deal with multibond reactions without having to include high-energy diabatic states. The global transformation matrix to the new diabatic representation, called the spin-valence diabatic representation, is constructed as the product of channel-specific transformation matrices, each one taken as the product of an asymptotic transformation matrix and a scaling function that depends on ratios of the spin-orbit splitting and the valence splittings. Thus the underlying basis functions are recoupled into suitable diabatic basis functions in a manner that
Proton-driven spin diffusion in rotating solids via reversible and irreversible quantum dynamics
Veshtort, Mikhail; Griffin, Robert G.
2011-01-01
Proton-driven spin diffusion (PDSD) experiments in rotating solids have received a great deal of attention as a potential source of distance constraints in large biomolecules. However, the quantitative relationship between the molecular structure and observed spin diffusion has remained obscure due to the lack of an accurate theoretical description of the spin dynamics in these experiments. We start with presenting a detailed relaxation theory of PDSD in rotating solids that provides such a description. The theory applies to both conventional and radio-frequency-assisted PDSD experiments and extends to the non-Markovian regime to include such phenomena as rotational resonance (R2). The basic kinetic equation of the theory in the non-Markovian regime has the form of a memory function equation, with the role of the memory function played by the correlation function. The key assumption used in the derivation of this equation expresses the intuitive notion of the irreversible dissipation of coherences in macroscopic systems. Accurate expressions for the correlation functions and for the spin diffusion constants are given. The theory predicts that the spin diffusion constants governing the multi-site PDSD can be approximated by the constants observed in the two-site diffusion. Direct numerical simulations of PDSD dynamics via reversible Liouville-von Neumann equation are presented to support and compliment the theory. Remarkably, an exponential decay of the difference magnetization can be observed in such simulations in systems consisting of only 12 spins. This is a unique example of a real physical system whose typically macroscopic and apparently irreversible behavior can be traced via reversible microscopic dynamics. An accurate value for the spin diffusion constant can be usually obtained through direct simulations of PDSD in systems consisting of two 13C nuclei and about ten 1H nuclei from their nearest environment. Spin diffusion constants computed by this method
Immense Magnetic Response of Exciplex Light Emission due to Correlated Spin-Charge Dynamics
NASA Astrophysics Data System (ADS)
Wang, Yifei; Sahin-Tiras, Kevser; Harmon, Nicholas J.; Wohlgenannt, Markus; Flatté, Michael E.
2016-01-01
As carriers slowly move through a disordered energy landscape in organic semiconductors, tiny spatial variations in spin dynamics relieve spin blocking at transport bottlenecks or in the electron-hole recombination process that produces light. Large room-temperature magnetic-field effects (MFEs) ensue in the conductivity and luminescence. Sources of variable spin dynamics generate much larger MFEs if their spatial structure is correlated on the nanoscale with the energetic sites governing conductivity or luminescence such as in coevaporated organic blends within which the electron resides on one molecule and the hole on the other (an exciplex). Here, we show that exciplex recombination in blends exhibiting thermally activated delayed fluorescence produces MFEs in excess of 60% at room temperature. In addition, effects greater than 4000% can be achieved by tuning the device's current-voltage response curve by device conditioning. Both of these immense MFEs are the largest reported values for their device type at room temperature. Our theory traces this MFE and its unusual temperature dependence to changes in spin mixing between triplet exciplexes and light-emitting singlet exciplexes. In contrast, spin mixing of excitons is energetically suppressed, and thus spin mixing produces comparatively weaker MFEs in materials emitting light from excitons by affecting the precursor pairs. Demonstration of immense MFEs in common organic blends provides a flexible and inexpensive pathway towards magnetic functionality and field sensitivity in current organic devices without patterning the constituent materials on the nanoscale. Magnetic fields increase the power efficiency of unconditioned devices by 30% at room temperature, also showing that magnetic fields may increase the efficiency of the thermally activated delayed fluorescence process.
The dynamic critical properties of the spin-2 Ising model on a bilayer square lattice
NASA Astrophysics Data System (ADS)
Temizer, Ümüt; Yarar, Semih; Tülek, Mesimi
2016-05-01
The spin-2 Ising model is investigated for the ferromagnetic/ferromagnetic (FM/FM), antiferromagnetic/ferromagnetic (AFM/FM) and antiferromagnetic/antiferromagnetic (AFM/AFM) interactions on the two-layer square lattice by using the Glauber-type stochastic dynamics. The system is in contact with a heat bath at temperature T, and the exchange of energy with the heat bath occurs via one-spin flip. By employing the Master equation and Glauber transition rates, the dynamic equations of the system are obtained. These equations are solved by using the numerical methods. First, we investigate the average order parameters as a function of the time to find the phases in the system. Then, the temperature-dependence of the dynamic order parameters is examined to obtain the dynamic phase transition temperatures. The dynamic phase diagrams are presented on the different planes. According to the values of the system parameters, a variety of dynamic critical points such as tricritical point, triple point, quadruple point, critical end point, double critical end point, zero-temperature critical point, multicritical point and tetracritical point are obtained. The reentrant behavior is seen in the system for the AFM/AFM interaction. Finally, we also investigate the influence of the oscillating field frequency on the dynamic phase diagrams in detail.
Thompson, Andrew R; Binder, Benjamin P; McCaffrey, Jesse E; Svensson, Bengt; Thomas, David D
2015-01-01
While EPR allows for the characterization of protein structure and function due to its exquisite sensitivity to spin label dynamics, orientation, and distance, these measurements are often limited in sensitivity due to the use of labels that are attached via flexible monofunctional bonds, incurring additional disorder and nanosecond dynamics. In this chapter, we present methods for using a bifunctional spin label (BSL) to measure muscle protein structure and dynamics. We demonstrate that bifunctional attachment eliminates nanosecond internal rotation of the spin label, thereby allowing the accurate measurement of protein backbone rotational dynamics, including microsecond-to-millisecond motions by saturation transfer EPR. BSL also allows for accurate determination of helix orientation and disorder in mechanically and magnetically aligned systems, due to the label's stereospecific attachment. Similarly, labeling with a pair of BSL greatly enhances the resolution and accuracy of distance measurements measured by double electron-electron resonance (DEER). Finally, when BSL is applied to a protein with high helical content in an assembly with high orientational order (e.g., muscle fiber or membrane), two-probe DEER experiments can be combined with single-probe EPR experiments on an oriented sample in a process we call BEER, which has the potential for ab initio high-resolution structure determination. PMID:26477249
Quench dynamics of a Bose-Einstein condensate under synthetic spin-orbit coupling
NASA Astrophysics Data System (ADS)
Deng, Tian-Shu; Zhang, Wei; Yi, Wei; Guo, Guang-Can
2016-05-01
We study the quench dynamics of a Bose-Einstein condensate under a Raman-assisted synthetic spin-orbit coupling. To model the dynamical process, we adopt a self-consistent Bogoliubov approach, which is equivalent to applying the time-dependent Bogoliubov-de Gennes equations. We investigate the dynamics of the condensate fraction as well as the momentum distribution of the Bose gas following a sudden change of system parameters. Typically, the system evolves into a steady state in the long-time limit, which features an oscillating momentum distribution and a stationary condensate fraction. We investigate how different quench parameters such as the inter- and intraspecies interactions and the spin-orbit-coupling parameters affect the condensate fraction in the steady state. Furthermore, we find that the time average of the oscillatory momentum distribution in the long-time limit can be described by a generalized Gibbs ensemble with two branches of momentum-dependent Gibbs temperatures. Our study is relevant to the experimental investigation of dynamical processes in a spin-orbit-coupled Bose-Einstein condensate.
Quantum Dynamics of Many-body Spin Chains Using Atomic Ions
NASA Astrophysics Data System (ADS)
Senko, Crystal
2014-05-01
Quantum simulation, a field in which well-controlled quantum systems are used to study many-body physics that would otherwise be challenging to model, has undergone a great deal of progress in recent years. In particular, trapped ions have proven an excellent platform for simulating quantum magnetism, with their long-lived coherence times, tunable spin-spin interactions mediated by optical dipole forces, and ease of individual readout. The manipulation of more than 10 spins is now routine and has allowed the study of dynamics that will be difficult to simulate classically in larger systems, such as spectroscopy of excitation energies (arXiv:1401.5751) and the spread of spin correlations in a system with long-range interactions (arXiv:1401.5088). In the near future, we expect to apply these techniques to the study of a variety of phenomena such as prethermalization in an isolated quantum system, and to upgrade the apparatus so as to handle many tens of spins, a system size well beyond what is classically calculable. This work is supported by grants from the U.S. Army Research Office with funding from the DARPA OLE program, IARPA, and the MURI program; and the NSF Physics Frontier Center at JQI.
Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO4
Toft-Petersen, Rasmus; Reehuis, Manfred; Jensen, Thomas B. S.; Andersen, Niels H.; Li, Jiying; Le, Manh Duc; Laver, Mark; Niedermayer, Christof; Klemke, Bastian; Lefmann, Kim; et al
2015-07-06
We report significant details of the magnetic structure and spin dynamics of LiFePO4 obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis. In addition, we find a significant spin-canting component along c. Furthermore, the possible causes of these components are discussed, and their significance for the magnetoelectric effect is analyzed. Inelastic neutron scattering along the three principal directions reveals a highly anisotropic hard plane consistent with earlier susceptibility measurements. While using a spin Hamiltonian, we showmore » that the spin dimensionality is intermediate between XY- and Ising-like, with an easy b axis and a hard c axis. As a result, it is shown that both next-nearest neighbor exchange couplings in the bc plane are in competition with the strongest nearest neighbor coupling.« less
Interacting spins in a cavity: Finite-size effects and symmetry-breaking dynamics
NASA Astrophysics Data System (ADS)
Gammelmark, Søren; Mølmer, Klaus
2012-04-01
We calculate the ground state and simulate the dynamics of a finite chain of spins with Ising nearest-neighbor interactions and a Dicke collective spin interaction with a single-mode cavity field. We recover the signatures of first- and second-order phase transitions predicted by mean-field theory, and for small chains, we find significant and nontrivial finite-size effects. Below the first-order phase transition, even quite large spin chains of 30-40 spins give rise to a mean photon number and number fluctuations significantly above the mean-field vacuum result. Near the second-order phase critical point, our calculations reveal photon number fluctuations that grow beyond Poisson statistics with the size of the spin chain. We simulate the stochastic evolution of the system when the cavity output field is subject to homodyne detection. For an initial state close to the first-order phase-transition the random character of the measurement process causes a measurement-induced symmetry breaking in the system. This symmetry breaking occurs on the time scale needed for an observer to gather sufficient information to distinguish between the two possible (mean-field) symmetry-broken states.
Imaging Spin Dynamics on the Nanoscale using X-Ray Microscopy
NASA Astrophysics Data System (ADS)
Stoll, Hermann; Noske, Matthias; Weigand, Markus; Richter, Kornel; Krüger, Benjamin; Reeve, Robert; Hänze, Max; Adolff, Christian; Stein, Falk-Ulrich; Meier, Guido; Kläui, Mathias; Schütz, Gisela
2015-04-01
The dynamics of emergent magnetic quasiparticles, such as vortices, domain walls, and bubbles are studied by scanning transmission x-ray microscopy (STXM), combining magnetic (XMCD) contrast with about 25 nm lateral resolution as well as 70 ps time resolution. Essential progress in the understanding of magnetic vortex dynamics is achieved by vortex core reversal observed by sub-GHz excitation of the vortex gyromode, either by ac magnetic fields or spin transfer torque. The basic switching scheme for this vortex core reversal is the generation of a vortex-antivortex pair. Much faster vortex core reversal is obtained by exciting azimuthal spin wave modes with (multi-GHz) rotating magnetic fields or orthogonal monopolar field pulses in x and y direction, down to 45 ps in duration. In that way unidirectional vortex core reversal to the vortex core 'down' or 'up' state only can be achieved with switching times well below 100 ps. Coupled modes of interacting vortices mimic crystal properties. The individual vortex oscillators determine the properties of the ensemble, where the gyrotropic mode represents the fundamental excitation. By self-organized state formation we investigate distinct vortex core polarization configurations and understand these eigenmodes in an extended Thiele model. Analogies with photonic crystals are drawn. Oersted fields and spin-polarized currents are used to excite the dynamics of domain walls and magnetic bubbles. From the measured phase and amplitude of the displacement of domain walls we deduce the size of the non-adiabatic spin-transfer torque. For sensing applications, the displacement of domain walls is studied and a direct correlation between domain wall velocity and spin structure is found. Finally the synchronous displacement of multiple domain walls using perpendicular field pulses is demonstrated as a possible paradigm shift for magnetic memory and logic applications.
Wigner, E.P.; Ohlinger, L.E.; Young, G.J.; Weinberg, A.M.
1959-02-17
Radiation shield construction is described for a nuclear reactor. The shield is comprised of a plurality of steel plates arranged in parallel spaced relationship within a peripheral shell. Reactor coolant inlet tubes extend at right angles through the plates and baffles are arranged between the plates at right angles thereto and extend between the tubes to create a series of zigzag channels between the plates for the circulation of coolant fluid through the shield. The shield may be divided into two main sections; an inner section adjacent the reactor container and an outer section spaced therefrom. Coolant through the first section may be circulated at a faster rate than coolant circulated through the outer section since the area closest to the reactor container is at a higher temperature and is more radioactive. The two sections may have separate cooling systems to prevent the coolant in the outer section from mixing with the more contaminated coolant in the inner section.
Dynamics of open quantum spin systems: An assessment of the quantum master equation approach.
Zhao, P; De Raedt, H; Miyashita, S; Jin, F; Michielsen, K
2016-08-01
Data of the numerical solution of the time-dependent Schrödinger equation of a system containing one spin-1/2 particle interacting with a bath of up to 32 spin-1/2 particles is used to construct a Markovian quantum master equation describing the dynamics of the system spin. The procedure of obtaining this quantum master equation, which takes the form of a Bloch equation with time-independent coefficients, accounts for all non-Markovian effects inasmuch the general structure of the quantum master equation allows. Our simulation results show that, with a few rather exotic exceptions, the Bloch-type equation with time-independent coefficients provides a simple and accurate description of the dynamics of a spin-1/2 particle in contact with a thermal bath. A calculation of the coefficients that appear in the Redfield master equation in the Markovian limit shows that this perturbatively derived equation quantitatively differs from the numerically estimated Markovian master equation, the results of which agree very well with the solution of the time-dependent Schrödinger equation. PMID:27627265
NASA Astrophysics Data System (ADS)
Gerving, C. S.; Hoang, T. M.; Land, B. J.; Anquez, M.; Hamley, C. D.; Chapman, M. S.
2012-11-01
A pendulum prepared perfectly inverted and motionless is a prototype of unstable equilibrium and corresponds to an unstable hyperbolic fixed point in the dynamical phase space. Here, we measure the non-equilibrium dynamics of a spin-1 Bose-Einstein condensate initialized as a minimum uncertainty spin-nematic state to a hyperbolic fixed point of the phase space. Quantum fluctuations lead to non-linear spin evolution along a separatrix and non-Gaussian probability distributions that are measured to be in good agreement with exact quantum calculations up to 0.25s. At longer times, atomic loss due to the finite lifetime of the condensate leads to larger spin oscillation amplitudes, as orbits depart from the separatrix. This demonstrates how decoherence of a many-body system can result in apparent coherent behaviour. This experiment provides new avenues for studying macroscopic spin systems in the quantum limit and for investigations of important topics in non-equilibrium quantum dynamics.
Mchaourab, Hassane S.; Steed, P. Ryan; Kazmier, Kelli
2011-01-01
Trapping membrane proteins in the confines of a crystal lattice obscures dynamic modes essential for interconversion between multiple conformations in the functional cycle. Moreover, lattice forces could conspire with detergent solubilization to stabilize a minor conformer in an ensemble thus confounding mechanistic interpretation. Spin labeling in conjunction with electron paramagnetic resonance (EPR) spectroscopy offers an exquisite window into membrane protein dynamics in the native–like environment of a lipid bilayer. Systematic application of spin labeling and EPR identifies sequence-specific secondary structures, defines their topology and their packing in the tertiary fold. Long range distance measurements (60-80Å) between pairs of spin labels enable quantitative analysis of equilibrium dynamics and triggered conformational changes. This review highlights the contribution of spin labeling to bridging structure and mechanism. Efforts to develop methods for determining structures from EPR restraints and to increase sensitivity and throughput promise to expand spin labeling applications in membrane protein structural biology. PMID:22078555
Dynamic shape effect in {sup 126}Ba at low spin
Dewald, A.; Weil, D.; Kruecken, R.; Kuehn, R.; Peusquens, R.; Tiesler, H.; Vogel, O.; Zell, K.O.; von Brentano, P.; Bazzacco, D.; Rossi-Alvarez, C.; Pavan, P.; DeAcuna, D.; De Angelis, G.; De Poli, M. ||
1996-11-01
Lifetimes of excited states in {sup 126}Ba have been measured with high precision by means of the GASP spectrometer using the coincidence recoil distance technique. The reaction {sup 100}Mo({sup 30}Si,4{ital n}) {sup 126}Ba at a beam energy of 130 MeV was used. The data were analyzed with the differential decay-curve method (DDCM). The obtained transition quadrupole moments disagree with the predictions of the asymmetric rotor model (ARM), the interacting boson model (IBM), and the general collective model (GCM). They give evidence for a sudden dynamic shape change in {sup 126}Ba between the 4{sup +} and 10{sup +} levels of the ground-state band. {copyright} {ital 1996 The American Physical Society.}
Dynamical thermal conductivity of the spin Lieb lattice
NASA Astrophysics Data System (ADS)
Yarmohammadi, Mohsen
2016-05-01
In the ferromagnetic insulator with the Dzyaloshinskii-Moriya interaction (DMI), we have theoretically investigated the dynamical thermal conductivity (DTC). In other words, we have investigated the frequency dependence of thermal conductivity, κ, of the Lieb lattice, a face-centered square lattice, subjected to a time dependence temperature gradient. Using linear response theory and Green's function approach, DTC has been obtained in the context of Heisenberg Hamiltonian. At low frequencies, DTC is found to be monotonically increasing with DMI strength (DMIS), temperature and next-nearest-neighbor (NNN) coupling. Also we have found that DTC includes a peak for different values of temperature, DMIS and NNN coupling. Furthermore we study the temperature dependence of thermal conductivity of Lieb lattice for different values of DMIS, NNN coupling and external magnetic filed. We witness a decrease in DTC with temperature due to the quantum effects in the system.
Dynamic spin filtering at the Co/Alq3 interface mediated by weakly coupled second layer molecules.
Droghetti, Andrea; Thielen, Philip; Rungger, Ivan; Haag, Norman; Großmann, Nicolas; Stöckl, Johannes; Stadtmüller, Benjamin; Aeschlimann, Martin; Sanvito, Stefano; Cinchetti, Mirko
2016-01-01
Spin filtering at organic-metal interfaces is often determined by the details of the interaction between the organic molecules and the inorganic magnets used as electrodes. Here we demonstrate a spin-filtering mechanism based on the dynamical spin relaxation of the long-living interface states formed by the magnet and weakly physisorbed molecules. We investigate the case of Alq3 on Co and, by combining two-photon photoemission experiments with electronic structure theory, show that the observed long-time spin-dependent electron dynamics is driven by molecules in the second organic layer. The interface states formed by physisorbed molecules are not spin-split, but acquire a spin-dependent lifetime, that is the result of dynamical spin-relaxation driven by the interaction with the Co substrate. Such spin-filtering mechanism has an important role in the injection of spin-polarized carriers across the interface and their successive hopping diffusion into successive molecular layers of molecular spintronics devices. PMID:27578395
Yamamura, Takafumi; Kiba, Takayuki; Yang, Xiaojie; Takayama, Junichi; Subagyo, Agus; Sueoka, Kazuhisa; Murayama, Akihiro
2014-09-07
The growth-temperature dependence of the optical spin-injection dynamics in self-assembled quantum dots (QDs) of In{sub 0.5}Ga{sub 0.5}As was studied by increasing the sheet density of the dots from 2 × 10{sup 10} to 7 × 10{sup 10} cm{sup −2} and reducing their size through a decrease in growth temperature from 500 to 470 °C. The circularly polarized transient photoluminescence (PL) of the resulting QD ensembles was analyzed after optical excitation of spin-polarized carriers in GaAs barriers by using rate equations that take into account spin-injection dynamics such as spin-injection time, spin relaxation during injection, spin-dependent state-filling, and subsequent spin relaxation. The excitation-power dependence of the transient circular polarization of PL in the QDs, which is sensitive to the state-filling effect, was also examined. It was found that a systematic increase occurs in the degree of circular polarization of PL with decreasing growth temperature, which reflects the transient polarization of exciton spin after spin injection. This is attributed to strong suppression of the filling effect for the majority-spin states as the dot-density of the QDs increases.
Spin-lattice dynamics simulation of external field effect on magnetic order of ferromagnetic iron
Chui, C. P.; Zhou, Yan
2014-03-15
Modeling of field-induced magnetization in ferromagnetic materials has been an active topic in the last dozen years, yet a dynamic treatment of distance-dependent exchange integral has been lacking. In view of that, we employ spin-lattice dynamics (SLD) simulations to study the external field effect on magnetic order of ferromagnetic iron. Our results show that an external field can increase the inflection point of the temperature. Also the model provides a better description of the effect of spin correlation in response to an external field than the mean-field theory. An external field has a more prominent effect on the long range magnetic order than on the short range counterpart. Furthermore, an external field allows the magnon dispersion curves and the uniform precession modes to exhibit magnetic order variation from their temperature dependence.
An efficient numerical method for computing dynamics of spin F = 2 Bose-Einstein condensates
Wang Hanquan
2011-07-01
In this paper, we extend the efficient time-splitting Fourier pseudospectral method to solve the generalized Gross-Pitaevskii (GP) equations, which model the dynamics of spin F = 2 Bose-Einstein condensates at extremely low temperature. Using the time-splitting technique, we split the generalized GP equations into one linear part and two nonlinear parts: the linear part is solved with the Fourier pseudospectral method; one of nonlinear parts is solved analytically while the other one is reformulated into a matrix formulation and solved by diagonalization. We show that the method keeps well the conservation laws related to generalized GP equations in 1D and 2D. We also show that the method is of second-order in time and spectrally accurate in space through a one-dimensional numerical test. We apply the method to investigate the dynamics of spin F = 2 Bose-Einstein condensates confined in a uniform/nonuniform magnetic field.
The dynamics of spin stabilized spacecraft with movable appendages, part 2
NASA Technical Reports Server (NTRS)
Bainum, P. M.
1976-01-01
The dynamics and stability of a spin stabilized spacecraft with a hinged appendage system are treated analytically and numerically. The hinged system consists of a central hub with masses attached to (assumed) massless booms of fixed length whose orientation relative to the main part can change. The general three dimensional deployment dynamics of such a hinged system is considered without any restriction on the location of the hinge points. The equations of motion for the hinged system, with viscous damping at both hinge points, are linearized about the nominal equilibrium position where the booms are orthogonal to the nominal spin axis for the case of two dimensional and three dimensional motion. Analytic stability criteria are obtained from the necessary condition on the sign of all the coefficients in the system characteristic equation.
Rapid 3D dynamic arterial spin labeling with a sparse model-based image reconstruction.
Zhao, Li; Fielden, Samuel W; Feng, Xue; Wintermark, Max; Mugler, John P; Meyer, Craig H
2015-11-01
Dynamic arterial spin labeling (ASL) MRI measures the perfusion bolus at multiple observation times and yields accurate estimates of cerebral blood flow in the presence of variations in arterial transit time. ASL has intrinsically low signal-to-noise ratio (SNR) and is sensitive to motion, so that extensive signal averaging is typically required, leading to long scan times for dynamic ASL. The goal of this study was to develop an accelerated dynamic ASL method with improved SNR and robustness to motion using a model-based image reconstruction that exploits the inherent sparsity of dynamic ASL data. The first component of this method is a single-shot 3D turbo spin echo spiral pulse sequence accelerated using a combination of parallel imaging and compressed sensing. This pulse sequence was then incorporated into a dynamic pseudo continuous ASL acquisition acquired at multiple observation times, and the resulting images were jointly reconstructed enforcing a model of potential perfusion time courses. Performance of the technique was verified using a numerical phantom and it was validated on normal volunteers on a 3-Tesla scanner. In simulation, a spatial sparsity constraint improved SNR and reduced estimation errors. Combined with a model-based sparsity constraint, the proposed method further improved SNR, reduced estimation error and suppressed motion artifacts. Experimentally, the proposed method resulted in significant improvements, with scan times as short as 20s per time point. These results suggest that the model-based image reconstruction enables rapid dynamic ASL with improved accuracy and robustness. PMID:26169322
Obaid, Rana; Kinzel, Daniel; Oppel, Markus González, Leticia
2014-10-28
Despite the concept of nuclear spin isomers (NSIs) exists since the early days of quantum mechanics, only few approaches have been suggested to separate different NSIs. Here, a method is proposed to discriminate different NSIs of a quinodimethane derivative using its electronic excited state dynamics. After electronic excitation by a laser field with femtosecond time duration, a difference in the behavior of several quantum mechanical operators can be observed. A pump-probe experimental approach for separating these different NSIs is then proposed.
Magnetic soft x-ray microscopy-imaging fast spin dynamics inmagnetic nanostructures
Fischer, Peter; Kim, Dong-Hyun; Mesler, Brooke L.; Chao, Weilun; Sakdinawat, Anne E.; Anderson, Erik H.
2007-06-01
Magnetic soft X-ray microscopy combines 15nm spatial resolution with 70ps time resolution and elemental sensitivity. Fresnel zone plates are used as X-ray optics and X-ray magnetic circular dichroism serves as magnetic contrast mechanism. Thus scientifically interesting and technologically relevant low dimensional nanomagnetic systems can be imaged at fundamental length and ultrafast time scales in a unique way. Studies include magnetization reversal in magnetic multilayers, nanopatterned systems, vortex dynamics in nanoelements and spin current induced phenomena.
The dynamics of diluted Ho spin ice Ho2-xYxTi2O7 studied byneutron spin echo spectroscopy
Ehlers, G.; Gardner, J.S.; Booth, C.H.; Daniel, M.; Kam, K.C.; Cheetham, A.K.; Antonio, D.; Brooks, H.E.; Cornelius, A.L.; Bramwell,S.T.; Lago, J.; Haussler, W.; Rosov, N.
2006-02-27
We have studied the spin relaxation in diluted spin ice Ho{sub 2-x} Y{sub x} Ti{sub 2}O{sub 7} by means of neutron spin echo spectroscopy. Remarkably, the geometrical frustration is not relieved by doping with non-magnetic Y, and the dynamics of the freezing is unaltered in the spin echo time window up to x {approx_equal} 1.6. At higher doping with non-magnetic Y (x {ge} 1.6) a new relaxation process at relatively high temperature (up to at least T {approx_equal} 55 K) appears which is more than 10 times faster than the thermally activated main relaxation process. We find evidence that over the whole range of composition all Ho spins participate in the dynamics. These results are compared to a.c. susceptibility measurements of the diluted Ho and Dy spin ice systems. X-ray absorption fine structure (EXAFS) spectra and x-ray diffraction show that the samples are structurally well ordered.
Bioengineering Spin-Offs from Dynamical Systems Theory
NASA Astrophysics Data System (ADS)
Collins, J. J.
1997-03-01
Recently, there has been considerable interest in applying concepts and techniques from dynamical systems and statistical physics to physiological systems. In this talk, we present work dealing which two active topics in this area: stochastic resonance and (2) chaos control. Stochastic resonance is a phenomenon wherein the response of nonlinear system to a weak input signal is optimally enhanced by the presence of a particular level of noise. Here we demonstrate that noise-based techniques can be used to lower sensory detection thresholds in humans. We discuss how from a bioengineering and clinical standpoint, these developments may be particularly relevant for individuals with elevated sensory thresholds, such as older adults and patients with peripheral neuropathy. Chaos control techniques have been applied to a wide range of experimental systems, including biological preparations. The application of chaos control to biological systems has led to speculations that these methods may be clinically useful. Here we demonstrate that the principles of chaos control can be utilized to stabilize underlying unstable periodic orbits in non-chaotic biological systems. We discuss how from a bioengineering and clinical standpoint, these developments may be important for suppressing or eliminating certain types of cardiac arrhythmias.
New Dynamic Spin Rig Capabilities Used to Determine Rotating Blade Dynamics
NASA Technical Reports Server (NTRS)
Provenza, Andrew J.
2004-01-01
The Dynamic Spin Rig Facility at the NASA Glenn Research Center is used to determine the structural response of rotating engine components without the effects of aerodynamic loading. Recently, this rig's capabilities were enhanced through the replacement of grease-lubricated ball bearings with magnetic bearings. Magnetic bearings offer a number of advantages--the most important here being that they not only fully support the rotor system, but excite it as well. Three magnetic bearings support the rotor and provide five axes of controlled motion: an x- and y-axis translation at each of two radial bearings and a z-axis translation in the vertical or axial direction. Sinusoidal excitation (most commonly used) can be imparted on the rotor through the radial magnetic bearings in either a fixed or rotating frame of reference. This excitation is added directly to the magnetic bearing control output. Since the rotor is fully levitated, large translations and rotations of the rotor system can be achieved. Some of the capabilities of this excitation system were determined and reported. The accelerations obtained at the tip of a titanium flat plate test article versus the swept sine excitation sent to both radial bearings in phase and perpendicular to the plane containing the two blades are shown. Recent tests required the excitation of fundamental bending and torsional blade resonances at rotor speeds up to 10,000 rpm. Successful fixed synchronous rotation of the excitation signal provided the best detectable blade resonant vibrations at excitation frequencies up to 1100 Hz for the particular blades of interest. A noncontacting laser measurement system was used to collect blade-tip motions. From these data, the amplitude and frequency of the motion could be determined as well as the blade damping properties. Damping could be determined using two methods: (1) free decay and (2) curve fitting the vibration amplitude as a function of frequency in and around the resonance of
RVB signatures in the spin dynamics of the square-lattice Heisenberg antiferromagnet
NASA Astrophysics Data System (ADS)
Ghioldi, E. A.; Gonzalez, M. G.; Manuel, L. O.; Trumper, A. E.
2016-03-01
We investigate the spin dynamics of the square-lattice spin-\\frac{1}{2} Heisenberg antiferromagnet by means of an improved mean-field Schwinger boson calculation. By identifying both, the long-range Néel and the RVB-like components of the ground state, we propose an educated guess for the mean-field magnetic excitation consisting on a linear combination of local and bond spin flips to compute the dynamical structure factor. Our main result is that when this magnetic excitation is optimized in such a way that the corresponding sum rule is fulfilled, we recover the low- and high-energy spectral weight features of the experimental spectrum. In particular, the anomalous spectral weight depletion at (π,0) found in recent inelastic neutron scattering experiments can be attributed to the interference of the triplet bond excitations of the RVB component of the ground state. We conclude that the Schwinger boson theory seems to be a good candidate to adequately interpret the dynamic properties of the square-lattice Heisenberg antiferromagnet.
Spin Dynamics of Kelvin's Pebbles, Jellett's Eggs, and Shiva's Lingam Stones
NASA Astrophysics Data System (ADS)
Brecher, Kenneth
2015-04-01
Study of the problem of the rise of the center of mass (COM) of spinning objects is said to have begun in the late nineteenth century. These early mathematical treatments aimed to explain the motion of the newly invented and patented ``tippe top.'' This semi-spheroidal top will invert when spun on a smooth surface while raising its COM. Because of the importance of friction in their dynamics, such non-holonomic systems are not readily amenable to analytic treatment, or of intuitive understanding. In notes written in 1844 - before the invention of the tippe top - Lord Kelvin (William Thomson) discussed the problem of the rising COM of spinning objects. He experimented with both oblate and prolate ellipsoidal pebbles, but did not publish a complete theoretical treatment of the problem. J. H. Jellett, in his 1872 book ``Theory of Friction,'' provided a partial account of the related problem of the rise of the COM for an egg-shaped (ovoid) object, making use of a new (adiabatic) invariant of the motion that he devised. Naturally occurring prolate ellipsoidal ``Lingam stones'' from the Narmada River in India exhibit similar counter-intuitive dynamical behavior. When spun around its minor axis in a horizontal plane, a Lingam stone will stand erect and spin around its major axis in a vertical position. This presentation will explore the history and some of the experimental facts and theoretical ideas about the rotational dynamics of such physical objects.
NASA Astrophysics Data System (ADS)
Mahmud, K. W.; Tiesinga, E.
2013-08-01
We study the dynamics of spin-1 atoms in a periodic optical-lattice potential and an external magnetic field in a quantum quench scenario where we start from a superfluid ground state in a shallow lattice potential and suddenly raise the lattice depth. The time evolution of the nonequilibrium state shows collective collapse-and-revival oscillations of matter-wave coherence as well as oscillations in the spin populations. We show that the complex pattern of these two types of oscillations reveals details about the superfluid and magnetic properties of the initial many-body ground state. Furthermore, we show that the strengths of the spin-dependent and spin-independent atom-atom interactions can be deduced from the observations. The Hamiltonian that describes the physics of the final deep lattice not only contains two-body interactions but also effective multibody interactions, which arise due to virtual excitations to higher bands. We derive these effective spin-dependent three-body interaction parameters for spin-1 atoms and describe how spin mixing is affected. Spinor atoms are unique in the sense that multibody interactions are directly evident in the in situ number densities in addition to the momentum distributions. We treat both antiferromagnetic (e.g., 23Na) and ferromagnetic (e.g., 87Rb and 41K) condensates.
Inelastic neutron scattering studies of the spin and lattice dynamics in iron arsenide compounds.
Osborn, R.; Rosenkranz, S.; Goremychkin, E. A.; Christianson, A. D.
2009-03-20
Although neutrons do not couple directly to the superconducting order parameter, they have nevertheless played an important role in advancing our understanding of the pairing mechanism and the symmetry of the superconducting energy gap in the iron arsenide compounds. Measurements of the spin and lattice dynamics have been performed on non-superconducting 'parent' compounds based on the LaFeAsO ('1111') and BaFe{sub 2}As{sub 2} ('122') crystal structures, and on electron and hole-doped superconducting compounds, using both polycrystalline and single crystal samples. Neutron measurements of the phonon density-of-state, subsequently supported by single crystal inelastic X-ray scattering, are in good agreement with ab initio calculations, provided the magnetism of the iron atoms is taken into account. However, when combined with estimates of the electron-phonon coupling, the predicted superconducting transition temperatures are less than 1 K, making a conventional phononic mechanism for superconductivity highly unlikely. Measurements of the spin dynamics within the spin density wave phase of the parent compounds show evidence of strongly dispersive spin waves with exchange interactions consistent with the observed magnetic order and a large anisotropy gap. Antiferromagnetic fluctuations persist in the normal phase of the superconducting compounds, but they are more diffuse. Below T{sub c}, there is evidence in three '122' compounds that these fluctuations condense into a resonant spin excitation at the antiferromagnetic wavevector with an energy that scales with T{sub c}. Such resonances have been observed in the high-T{sub c} copper oxides and a number of heavy fermion superconductors, where they are considered to be evidence of d-wave symmetry. In the iron arsenides, they also provide evidence of unconventional superconductivity, but a comparison with ARPES and other measurements, which indicate that the gaps are isotropic, suggests that the symmetry is more likely
Inelastic Neutron Scattering Studies of the Spin and Lattice Dynamics inIron Arsenide Compounds
Christianson, Andrew D; Osborn, R.; Rosenkranz, Stephen; Goremychkin, E. A.
2009-01-01
Although neutrons do not couple directly to the superconducting order parameter, they have nevertheless played an important role in advancing our understanding of the pairing mechanism and the symmetry of the superconducting energy gap in the iron arsenide compounds. Measurements of the spin and lattice dynamics have been performed on non-superconducting 'parent' compounds based on the LaFeAsO ('1111') and BaFe{sub 2}As{sub 2} ('122') crystal structures, and on electron and hole-doped superconducting compounds, using both polycrystalline and single crystal samples. Neutron measurements of the phonon density-of-state, subsequently supported by single crystal inelastic X-ray scattering, are in good agreement with ab initio calculations, provided the magnetism of the iron atoms is taken into account. However, when combined with estimates of the electron-phonon coupling, the predicted superconducting transition temperatures are less than 1 K, making a conventional phononic mechanism for superconductivity highly unlikely. Measurements of the spin dynamics within the spin density wave phase of the parent compounds show evidence of strongly dispersive spin waves with exchange interactions consistent with the observed magnetic order and a large anisotropy gap. Antiferromagnetic fluctuations persist in the normal phase of the superconducting compounds, but they are more diffuse. Below T{sub c}, there is evidence in three '122' compounds that these fluctuations condense into a resonant spin excitation at the antiferromagnetic wavevector with an energy that scales with T{sub c}. Such resonances have been observed in the high-T{sub c} copper oxides and a number of heavy fermion superconductors, where they are considered to be evidence of d-wave symmetry. In the iron arsenides, they also provide evidence of unconventional superconductivity, but a comparison with ARPES and other measurements, which indicate that the gaps are isotropic, suggests that the symmetry is more likely
Time-quantified Monte Carlo algorithm for interacting spin array micromagnetic dynamics
NASA Astrophysics Data System (ADS)
Cheng, X. Z.; Jalil, M. B. A.; Lee, Hwee Kuan
2006-06-01
In this paper, we reexamine the validity of using time-quantified Monte Carlo (TQMC) method [Phys. Rev. Lett. 84, 163 (2000); 96, 067208 (2006)] in simulating the stochastic dynamics of interacting magnetic nanoparticles. The Fokker-Planck coefficients corresponding to both TQMC and the Langevin dynamical equation (Landau-Lifshitz-Gilbert, LLG) are derived and compared in the presence of interparticle interactions. The time quantification factor is obtained and justified. Numerical verification is shown by using TQMC and Langevin methods in analyzing spin-wave dispersion in a linear array of magnetic nanoparticles.
Domain wall dynamics in a spin-reorientation transition system Au/Co/Au
Roy, Sujoy; Seu, Keoki; Turner, Joshua J.; Park, Sungkyun; Kevan, Steve; Falco, Charles M.
2009-05-14
We report measurements of domain wall dynamics in an ultrathin Au/Co/Au system that exhibits a spin reorientation phase transition as a function of temperature.The domain walls exhibit cooperative motion throughout the temperature range of 150 - 300 K. The decay times were found to exhibit a maximum at the transition temperature. The slowdown has been explained as due to formation of a double well in the energy landscape by the different competing interactions. Our results show that the complex, slow dynamics can provide a more fundamental understanding of magnetic phase transitions.
Probing dynamics of fusion reactions through cross-section and spin distribution measurement
NASA Astrophysics Data System (ADS)
Kaur, Maninder; Behera, B. R.; Singh, Gulzar; Singh, Varinderjit; Madhavan, N.; Muralithar, S.; Nath, S.; Gehlot, J.; Mohanto, G.; Mukul, Ish; Siwal, D.; Thakur, M.; Kapoor, K.; Sharma, P.; Banerjee, T.; Jhingan, A.; Varughese, T.; Bala, Indu; Nayak, B. K.; Saxena, A.; Chatterjee, M. B.; Stevenson, P. D.
2016-05-01
Present work aims to explicate the effect of entrance channel mass asymmetry on fusion dynamics for the Compound Nucleus 80Sr populated through two different channels, 16O+64Zn and 32S+48Ti, using cross-section and spin distribution measurements as probes. The evaporation spectra studies for these systems, reported earlier indicate the presence of dynamical effects for mass symmetric 32S+48Ti system.The CCDEF and TDHF calculations have been performed for both the systems and an attempt has been made to explain the reported deviations in the α-particle spectrum for the mass symmetric system.
Davesne, V.; Gruber, M.; Miyamachi, T.; Da Costa, V.; Boukari, S.; Scheurer, F.; Joly, L.; Bowen, M.; Beaurepaire, E.; Ohresser, P.; Otero, E.; Choueikani, F.; Gaspar, A. B.; Real, J. A.; Wulfhekel, W.
2013-08-21
The dynamics of the soft x-ray induced excited spin state trapping (SOXIESST) effect of Fe(phen){sub 2}(NCS){sub 2} (Fe-phen) powder have been investigated by x-ray absorption spectroscopy (XAS) using the total electron yield method, in a wide temperature range. The low-spin (LS) state is excited into the metastable high-spin (HS) state at a rate that depends on the intensity of the x-ray illumination it receives, and both the temperature and the intensity of the x-ray illumination will affect the maximum HS proportion that is reached. We find that the SOXIESST HS spin state transforms back to the LS state at a rate that is similar to that found for the light induced excited spin state trapping (LIESST) effect. We show that it is possible to use the SOXIESST effect in combination with the LIESST effect to investigate the influence of cooperative behavior on the dynamics of both effects. To investigate the impact of molecular cooperativity, we compare our results on Fe-phen with those obtained for Fe([Me{sub 2}Pyrz]{sub 3}BH){sub 2} (Fe-pyrz) powder, which exhibits a similar thermal transition temperature but with a hysteresis. We find that, while the time constant of the dynamic is identical for both molecules, the SOXIESST effect is less efficient at exciting the HS state in Fe-pyrz than in Fe-phen.
NASA Astrophysics Data System (ADS)
Bertmer, Marko; Demco, Dan E.; Wang, Mingfei; Melian, Claudiu; Marcean-Chelcea, Ramona I.; Fechete, Radu; Baias, Maria; Blümich, Bernhard
2006-11-01
Segmental dynamic heterogeneity of short-chain grafted poly(dimethylsiloxane) (PDMS) on pyrogenic silica was investigated using 1H NMR spin-diffusion. A double-quantum dipolar filter was employed for selection of the interface (rigid) region. One-dimensional spin-diffusion equations were solved numerically for a space distribution of spin diffusivity D( x) of the mobile PDMS chains. The degree of heterogeneity can be quantified by the parameters of Gaussian and exponential diffusivity distribution functions which yield similar diffusivities. The rigid and mobile domain sizes and spin diffusivities were correlated with the PDMS chain length, the temperature, and 1H residual dipolar couplings.
Direct observation of magnetization dynamics generated by nanocontact spin-torque vortex oscillators
NASA Astrophysics Data System (ADS)
Keatley, P. S.; Sani, S. R.; Hrkac, G.; Mohseni, S. M.; Dürrenfeld, P.; Loughran, T. H. J.; Åkerman, J.; Hicken, R. J.
2016-08-01
Time-resolved scanning Kerr microscopy has been used to directly image the magnetization dynamics of nanocontact (NC) spin-torque vortex oscillators (STVOs) when phase locked to an injected microwave (rf) current. The Kerr images reveal free-layer magnetization dynamics that extend outside the NC footprint, where they cannot be detected electrically, but which are crucial to phase-lock STVOs that share common magnetic layers. For a single NC, dynamics were observed not only when the STVO frequency was fully locked to that of the rf current, but also for a partially locked state characterized by periodic changes in the core trajectory at the rf frequency. For a pair of NCs, we explore the correlation between the spatial character of injection-locked dynamics and the free-running spectra. Insight gained from these images may improve understanding of the conditions required for mutual phase locking of multiple STVOs, and hence enhanced microwave power emission.
NASA Astrophysics Data System (ADS)
Fong, C. F.; Ota, Y.; Harbord, E.; Iwamoto, S.; Arakawa, Y.
2016-03-01
Repeated injection of spin-polarized carriers in a quantum dot (QD) leads to the polarization of nuclear spins, a process known as dynamic nuclear spin polarization (DNP). Here, we report the observation of p-shell carrier assisted DNP in single QDs at zero external magnetic field. The nuclear field—measured by using the Overhauser shift of the singly charged exciton state of the QDs—continues to increase, even after the carrier population in the s-shell saturates. This is also accompanied by an abrupt increase in nuclear spin buildup time as p-shell emission overtakes that of the s shell. We attribute the observation to p-shell electrons strongly altering the nuclear spin dynamics in the QD, supported by numerical simulation results based on a rate equation model of coupling between electron and nuclear spin system. Dynamic nuclear spin polarization with p-shell carriers could open up avenues for further control to increase the degree of nuclear spin polarization in QDs.
Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer
NASA Astrophysics Data System (ADS)
Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J.; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent
2016-07-01
Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers.
Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer.
Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent
2016-01-01
Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers. PMID:27425776
Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer
Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent
2016-01-01
Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers. PMID:27425776
NASA Astrophysics Data System (ADS)
Onur, A. R.; de Jong, J. P.; O'Shea, D.; Reuter, D.; Wieck, A. D.; van der Wal, C. H.
2016-04-01
We experimentally demonstrate how coherent population trapping (CPT) for donor-bound electron spins in GaAs results in autonomous feedback that prepares stabilized states for the spin polarization of nuclei around the electrons. CPT was realized by excitation with two lasers to a bound-exciton state. Transmission studies of the spectral CPT feature on an ensemble of electrons directly reveal the statistical distribution of prepared nuclear-spin states. Tuning the laser driving from blue to red detuned drives a transition from one to two stable states. Our results have importance for ongoing research on schemes for dynamic nuclear-spin polarization, the central spin problem, and control of spin coherence.
Dependence of spin dynamics on in-plane magnetic field in AlGaN/GaN quantum wells
NASA Astrophysics Data System (ADS)
Lv, Meng; Yu, Guolin; Xu, Yonggang; Chang, Zhigang; Lin, Tie; Zhao, Degang; Dai, Ning; Chu, Junhao; Lockwood, D. J.
2015-12-01
We systematically investigate the weak antilocalization effect and the dependence of spin dynamics on the in-plane magnetic field for two Al x Ga1-x N/GaN quantum wells, in which these effects are dominated by the spin-orbit interaction originating from the structural inversion asymmetry and the bulk inversion asymmetry, respectively. By fitting the weak antilocalization magnetoconductance, the phase coherence time and spin-orbit scattering time are obtained. With the increase of in-plane magnetic fields, the phase coherence time decreases quadratically while the spin-orbit scattering time increases quadratically. We attribute these variations to the competition between the Zeeman splitting and the spin-orbit interaction. The comparison between systems dominated by structural inversion asymmetry and bulk inversion asymmetry in the in-plane magnetic field is also made. Our findings may provide clues to control the weak antilocalization effect and spin-orbit interaction via the in-plane field.
Density functional plus dynamical mean-field theory of the spin-crossover molecule Fe(phen)2(NCS)2
NASA Astrophysics Data System (ADS)
Chen, Jia; Millis, Andrew J.; Marianetti, Chris A.
2015-06-01
We study the spin-crossover molecule Fe(phen) 2(NCS) 2 using density functional theory (DFT) plus dynamical mean-field theory, which allows access to observables not attainable with traditional quantum chemical or electronic structure methods. The temperature dependent magnetic susceptibility, electron addition and removal spectra, and total energies are calculated and compared to experiment. We demonstrate that the proper quantitative energy difference between the high-spin and low-spin state, as well as reasonably accurate values of the magnetic susceptibility can be obtained when using reasonable interaction parameters. Comparisons to DFT and DFT+U calculations demonstrate that dynamical correlations are critical to the energetics of the low-spin state. Additionally, we elucidate the differences between DFT+U and spin density functional theory (SDFT) plus U methodologies, demonstrating that DFT+U can recover SDFT+U results for an appropriately chosen on-site exchange interaction.
Evidence of impurity and boundary effects on magnetic monopole dynamics in spin ice
NASA Astrophysics Data System (ADS)
Revell, H. M.; Yaraskavitch, L. R.; Mason, J. D.; Ross, K. A.; Noad, H. M. L.; Dabkowska, H. A.; Gaulin, B. D.; Henelius, P.; Kycia, J. B.
2013-01-01
Electrical resistance is a crucial and well-understood property of systems ranging from computer microchips to nerve impulse propagation in the human body. Here we study the motion of magnetic charges in spin ice and find that extra spins inserted in Dy2Ti2O7 trap magnetic monopole excitations and provide the first example of how defects in a spin-ice material obstruct the flow of monopoles--a magnetic version of residual resistance. We measure the time-dependent magnetic relaxation in Dy2Ti2O7 and show that it decays with a stretched exponential followed by a very slow long-time tail. In a Monte Carlo simulation governed by Metropolis dynamics we show that surface effects and a very low level of stuffed spins (0.30%)--magnetic Dy ions substituted for non-magnetic Ti ions--cause these signatures in the relaxation. In addition, we find evidence that the rapidly diverging experimental timescale is due to a temperature-dependent attempt rate proportional to the monopole density.
Dynamics of a coupled spin-vortex pair in dipolar spinor Bose-Einstein condensates
NASA Astrophysics Data System (ADS)
Li, Tiantian; Yi, Su; Zhang, Yunbo
2016-05-01
The collisional and magnetic field quench dynamics of a coupled spin-vortex pair in dipolar spinor Bose-Einstein condensates in a double-well potential are numerically investigated in the mean-field theory. Upon a sudden release of the potential barrier the two layers of condensates collide with each other in the trap center with the chirality of the vortex pair exchanged after each collision, showing the typical signature of in-phase collision for the parallel spin-vortex phase, and out-of-phase collision for the antiparallel phase. When quenching the transverse magnetic field, the vortex center in the single-layered condensate starts to make a helical motion with oval-shaped trajectories and the displacement of the center position is found to exhibit a damped simple harmonic oscillation with an intrinsic frequency and damping rate. The oscillation mode of the spin-vortex pair may be tuned by the initial magnetic field and the height of the Gaussian barrier; e.g., the gyrotropic motions for a parallel spin-vortex pair are out of sync with each other in the two layers, while those for the antiparallel pair exhibit a double-helix structure with the vortex centers moving opposite to each other with the same amplitude.
Minority-spin dynamics in the nonhomogeneous Ising model: Diverging time scales and exponents
NASA Astrophysics Data System (ADS)
Mullick, Pratik; Sen, Parongama
2016-05-01
We investigate the dynamical behavior of the Ising model under a zero-temperature quench with the initial fraction of up spins 0 ≤x ≤1 . In one dimension, the known results for persistence probability are verified; it shows algebraic decay for both up and down spins asymptotically with different exponents. It is found that the conventional finite-size scaling is valid here. In two dimensions, however, the persistence probabilities are no longer algebraic; in particular for x ≤0.5 , persistence for the up (minority) spins shows the behavior Pmin(t ) ˜t-γexp[-(t/τ ) δ] with time t , while for the down (majority) spins, Pmaj(t ) approaches a finite value. We find that the timescale τ diverges as (xc-x ) -λ, where xc=0.5 and λ ≃2.31 . The exponent γ varies as θ2 d+c0(xc-x ) β where θ2 d≃0.215 is very close to the persistence exponent in two dimensions; β ≃1 . The results in two dimensions can be understood qualitatively by studying the exit probability, which for different system size is found to have the form E (x ) =f [(x/-xc xc) L1 /ν] , with ν ≈1.47 . This result suggests that τ ˜Lz ˜ , where z ˜=λ/ν =1.57 ±0.11 is an exponent not explored earlier.
NASA Astrophysics Data System (ADS)
Asfaw, Abraham; Tyryshkin, Alexei; Lyon, Stephen
Global magnetic field fluctuations present significant challenges to pulsed electron spin resonance experiments on systems with long spin coherence times. We will discuss results from experiments in which we follow instantaneous changes in magnetic field by locking to the free induction decay of a proton NMR signal using a phase-locked loop. We extend conventional field-frequency locking techniques used in NMR to follow slow magnetic field drifts by using a modified Carr-Purcell-Meiboom-Gill (CPMG) pulse sequence in which the phase of the pi-pulses follows the phase of the proton spins at all times. Hence, we retain the ability of the CPMG pulse sequence to refocus local magnetic field inhomogeneities without refocusing global magnetic field fluctuations. In contrast with conventional field-frequency locking techniques, our experiments demonstrate the potential of this method to dynamically track global magnetic field fluctuations on timescales of about 2 seconds and with rates faster than a kHz. This frequency range covers the dominant noise frequencies in our electron spin resonance experiments as previously reported.
Improving the coherence properties of solid-state spin ensembles via optimized dynamical decoupling
NASA Astrophysics Data System (ADS)
Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.
2016-04-01
In this work, we optimize a dynamical decoupling (DD) protocol to improve the spin coherence properties of a dense ensemble of nitrogen-vacancy (NV) centers in diamond. Using liquid nitrogen-based cooling and DD microwave pulses, we increase the transverse coherence time T2 from ˜ 0.7 ms up to ˜ 30 ms. We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. After performing a detailed analysis of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the concatenated XY8 pulse sequences serves as the optimal control scheme for preserving an arbitrary spin state. Finally, we use the concatenated sequences to demonstrate an immediate improvement of the AC magnetic sensitivity up to a factor of two at 250 kHz. For future work, similar protocols may be used to increase coherence times up to NV-NV interaction time scales, a major step toward the creation of quantum collective NV spin states.
NASA Astrophysics Data System (ADS)
Venderbos, J. W. F.
2016-03-01
We study hexagonal spin-channel ("triplet") density waves with commensurate M -point propagation vectors. We first show that the three Q =M components of the singlet charge density and charge-current density waves can be mapped to multicomponent Q =0 nonzero angular momentum order in three dimensions (3D) with cubic crystal symmetry. This one-to-one correspondence is exploited to define a symmetry classification for triplet M -point density waves using the standard classification of spin-orbit coupled electronic liquid crystal phases of a cubic crystal. Through this classification we naturally identify a set of noncoplanar spin density and spin-current density waves: the chiral spin density wave and its time-reversal invariant analog. These can be thought of as 3 DL =2 and 4 spin-orbit coupled isotropic β -phase orders. In contrast, uniaxial spin density waves are shown to correspond to α phases. The noncoplanar triple-M spin-current density wave realizes a novel 2 D semimetal state with three flavors of four-component spin-momentum locked Dirac cones, protected by a crystal symmetry akin to nonsymmorphic symmetry, and sits at the boundary between a trivial and topological insulator. In addition, we point out that a special class of classical spin states, defined as classical spin states respecting all lattice symmetries up to global spin rotation, are naturally obtained from the symmetry classification of electronic triplet density waves. These symmetric classical spin states are the classical long-range ordered limits of chiral spin liquids.
Marry, Virginie; Dubois, Emmanuelle; Malikova, Natalie; Durand-Vidal, Serge; Longeville, Stéphane; Breu, Josef
2011-04-01
Within the wider context of water behavior in soils, and with a particular emphasis on clays surrounding underground radioactive waste packages, we present here the translational dynamics of water in clays in low hydrated states as studied by coupling molecular dynamics (MD) simulations and quasielastic neutron scattering experiments by neutron spin echo (NSE). A natural montmorillonite clay of interest is modeled by a synthetic clay which allows us to understand the determining parameters from MD simulations by comparison with the experimental values. We focus on temperatures between 300 and 350 K, i.e., the range relevant to the highlighted application. The activation energy Ea experimentally determined is 6.6 kJ/mol higher than that for bulk water. Simulations are in good agreement with experiments for the relevant set of conditions, and they give more insight into the origin of the observed dynamics. PMID:21381672
Nanocluster building blocks of artificial square spin ice: Stray-field studies of thermal dynamics
Pohlit, Merlin Porrati, Fabrizio; Huth, Michael; Müller, Jens
2015-05-07
We present measurements of the thermal dynamics of a Co-based single building block of an artificial square spin ice fabricated by focused electron-beam-induced deposition. We employ micro-Hall magnetometry, an ultra-sensitive tool to study the stray field emanating from magnetic nanostructures, as a new technique to access the dynamical properties during the magnetization reversal of the spin-ice nanocluster. The obtained hysteresis loop exhibits distinct steps, displaying a reduction of their “coercive field” with increasing temperature. Therefore, thermally unstable states could be repetitively prepared by relatively simple temperature and field protocols allowing one to investigate the statistics of their switching behavior within experimentally accessible timescales. For a selected switching event, we find a strong reduction of the so-prepared states' “survival time” with increasing temperature and magnetic field. Besides the possibility to control the lifetime of selected switching events at will, we find evidence for a more complex behavior caused by the special spin ice arrangement of the macrospins, i.e., that the magnetic reversal statistically follows distinct “paths” most likely driven by thermal perturbation.
Time-resolved x-ray imaging of magnetization dynamics in spin-transfer torque devices
Chembrolu, V.
2010-02-24
Time-resolved x-ray imaging techniques have recently demonstrated the capability to probe the magnetic switching of nanoscale devices. This technique has enabled, for example, the direct observation of the nonuniform intermediate states assumed by the magnetic free layer during reversal by a spin-polarized current. These experiments have shown an interesting size-dependent behavior associated with the motion of vortices to mediate the magnetization reversal which cannot be explained by the macrospin picture of spin-torque switching. In this paper we present both experimental and analytical results which show the origin of the complex switching behavior. We use time-resolved x-ray microscopy to further study the switching behavior of samples with 45{sup o} angle between the free and polarizing magnetic layers. A model is developed in terms of a linearized Landau-Lifshitz-Gilbert equation showing that the initial dynamics is dominated by the balance between the Oersted field and thermal fluctuations. The spin torque amplifies this dynamics, leading to a strong sensitivity to sample size, angle, and temperature. The model is in good agreement with current and previous experimental observations.
Tracking protein dynamics with photoconvertible Dendra2 on spinning disk confocal systems.
Woods, Elena; Courtney, Jane; Scholz, Dimitri; Hall, William W; Gautier, Virginie W
2014-12-01
Understanding the dynamic properties of cellular proteins in live cells and in real time is essential to delineate their function. In this context, we introduce the Fluorescence Recovery After Photobleaching-Photoactivation unit (Andor) combined with the Nikon Eclipse Ti E Spinning Disk (Andor) confocal microscope as an advantageous and robust platform to exploit the properties of the Dendra2 photoconvertible fluorescent protein (Evrogen) and analyse protein subcellular trafficking in living cells. A major advantage of the spinning disk confocal is the rapid acquisition speed, enabling high temporal resolution of cellular processes. Furthermore, photoconversion and imaging are less invasive on the spinning disk confocal as the cell exposition to illumination power is reduced, thereby minimizing photobleaching and increasing cell viability. We have tested this commercially available platform using experimental settings adapted to track the migration of fast trafficking proteins such as UBC9, Fibrillarin and have successfully characterized their differential motion between subnuclear structures. We describe here step-by-step procedures, with emphasis on cellular imaging parameters, to successfully perform the dynamic imaging and photoconversion of Dendra2-fused proteins at high spatial and temporal resolutions necessary to characterize the trafficking pathways of proteins. PMID:25186063
Kinematical and dynamical aspects of higher-spin bound-state equations in holographic QCD
de Téramond, Guy F.; Dosch, Hans Günter; Brodsky, Stanley J.
2013-04-01
In this paper we derive holographic wave equations for hadrons with arbitrary spin starting from an effective action in a higher-dimensional space asymptotic to anti–de Sitter (AdS) space. Our procedure takes advantage of the local tangent frame, and it applies to all spins, including half-integer spins. An essential element is the mapping of the higher-dimensional equations of motion to the light-front Hamiltonian, thus allowing a clear distinction between the kinematical and dynamical aspects of the holographic approach to hadron physics. Accordingly, the nontrivial geometry of pure AdS space encodes the kinematics, and the additional deformations of AdS space encode the dynamics, including confinement. It thus becomes possible to identify the features of holographic QCD, which are independent of the specific mechanisms of conformal symmetry breaking. In particular, we account for some aspects of the striking similarities and differences observed in the systematics of the meson and baryon spectra.
Analytical approach to the dynamics of facilitated spin models on random networks
NASA Astrophysics Data System (ADS)
Fennell, Peter G.; Gleeson, James P.; Cellai, Davide
2014-09-01
Facilitated spin models were introduced some decades ago to mimic systems characterized by a glass transition. Recent developments have shown that a class of facilitated spin models is also able to reproduce characteristic signatures of the structural relaxation properties of glass-forming liquids. While the equilibrium phase diagram of these models can be calculated analytically, the dynamics are usually investigated numerically. Here we propose a network-based approach, called approximate master equation (AME), to the dynamics of the Fredrickson-Andersen model. The approach correctly predicts the critical temperature at which the glass transition occurs. We also find excellent agreement between the theory and the numerical simulations for the transient regime, except in close proximity of the liquid-glass transition. Finally, we analytically characterize the critical clusters of the model and show that the departures between our AME approach and the Monte Carlo can be related to the large interface between blocked and unblocked spins at temperatures close to the glass transition.
Dynamics of Bound Monopoles in Artificial Spin Ice: How to Store Energy in Dirac Strings
NASA Astrophysics Data System (ADS)
Vedmedenko, E. Y.
2016-02-01
Dirac strings in spin ices are lines of reversed dipoles joining two quasiparticle excitations. These excitations behave as unbound emergent monopoles if the tension of Dirac strings vanishes. In this Letter, analytical and numerical analysis are used to study the dynamics of two-dimensional dipolar spin ices, artificially created analogs of bulk spin ice, in the regime of bound monopoles. It is shown that, in this regime, strings, rather than monopoles, are effective degrees of freedom explaining the finite-width band of Pauling states. A measurable prediction of path-time dependence of endpoints of a stretched and, then, released Dirac string is made and verified via simulations. It is shown that string dynamics is defined by the characteristic tension-to-mass ratio, which is determined by the fine structure constant and lattice dependent parameter. It is proposed to use string tension to achieve spontaneous magnetic currents. A concept of an energy storing device on the basis of this principle is proposed and illustrated by an experimental demonstration. A scheme of independent measurement at the nanoscale is proposed.
Dynamics of Bound Monopoles in Artificial Spin Ice: How to Store Energy in Dirac Strings.
Vedmedenko, E Y
2016-02-19
Dirac strings in spin ices are lines of reversed dipoles joining two quasiparticle excitations. These excitations behave as unbound emergent monopoles if the tension of Dirac strings vanishes. In this Letter, analytical and numerical analysis are used to study the dynamics of two-dimensional dipolar spin ices, artificially created analogs of bulk spin ice, in the regime of bound monopoles. It is shown that, in this regime, strings, rather than monopoles, are effective degrees of freedom explaining the finite-width band of Pauling states. A measurable prediction of path-time dependence of endpoints of a stretched and, then, released Dirac string is made and verified via simulations. It is shown that string dynamics is defined by the characteristic tension-to-mass ratio, which is determined by the fine structure constant and lattice dependent parameter. It is proposed to use string tension to achieve spontaneous magnetic currents. A concept of an energy storing device on the basis of this principle is proposed and illustrated by an experimental demonstration. A scheme of independent measurement at the nanoscale is proposed. PMID:26943555
Quantum spin dynamics and entanglement in systems with long-range interactions
NASA Astrophysics Data System (ADS)
Rey, Ana M.
One of the fundamental goals of modern quantum sciences is to learn how to control and manipulate non-equilibrium many-body systems and use them to make powerful and improved quantum devices, materials and technologies. However, out-of-equilibrium systems are complex, typically strongly correlated and entangled, and thus to model them we are in an urgent need of new methodologies. In this talk I will discuss new theoretical methods that we have developed to investigate emergent non-equilibrium phenomena in driven-dissipative spin systems interacting via long-range interactions. I will show we can capture the dynamics of correlations and entanglement in close systems and the interplay between dissipation and entanglement in open quantum systems including spin-boson models. As a specific application I will discuss the use of our methods to model the spin dynamics exhibited by arrays of trapped ions with controllable long-range interactions. I will show that our predictions are consistent with recent experimental measurements. I will also discuss new protocols to diagnostic and characterize entanglement based on well-established NMR protocols This work is supported by NSF, ARO, AFOSR-MURI, and NIST.
Development of fiber shields for engine containment. [mathematical models
NASA Technical Reports Server (NTRS)
Bristow, R. J.; Davidson, C. D.
1977-01-01
Tests were conducted in translational launchers and spin pits to generate empirical data used in the design of a Kevlar shield for containing engine burst debris. Methods are given for modeling the relationship of fragment characteristics to shielding requirements. The change in relative importance of shield mounting provisions as fragment energy is increased is discussed.
NASA Astrophysics Data System (ADS)
Arosio, Paolo; Corti, Maurizio; Mariani, Manuel; Orsini, Francesco; Bogani, Lapo; Caneschi, Andrea; Lago, Jorge; Lascialfari, Alessandro
2015-05-01
The spin dynamics of the molecular magnetic chain [Dy(hfac)3{NIT(C6H4OPh)}] were investigated by means of the Muon Spin Relaxation (μ+SR) technique. This system consists of a magnetic lattice of alternating Dy(III) ions and radical spins, and exhibits single-chain-magnet behavior. The magnetic properties of [Dy(hfac)3{NIT(C6H4OPh)}] have been studied by measuring the magnetization vs. temperature at different applied magnetic fields (H = 5, 3500, and 16500 Oe) and by performing μ+SR experiments vs. temperature in zero field and in a longitudinal applied magnetic field H = 3500 Oe. The muon asymmetry P(t) was fitted by the sum of three components, two stretched-exponential decays with fast and intermediate relaxation times, and a third slow exponential decay. The temperature dependence of the spin dynamics has been determined by analyzing the muon longitudinal relaxation rate λinterm(T), associated with the intermediate relaxing component. The experimental λinterm(T) data were fitted with a corrected phenomenological Bloembergen-Purcell-Pound law by using a distribution of thermally activated correlation times, which average to τ = τ0 exp(Δ/kBT), corresponding to a distribution of energy barriers Δ. The correlation times can be associated with the spin freezing that occurs when the system condenses in the ground state.
Dynamical correlation effects on structure factor of spin-polarized two-dimensional electron gas
Singh, Gurvinder; Moudgil, R. K.; Kumar, Krishan; Garg, Vinayak
2015-06-24
We report a theoretical study on static density structure factor S(q) of a spin-polarized two-dimensional electron gas over a wide range of electron number density r{sub s}. The electron correlations are treated within the dynamical version of the self-consistent mean-field theory of Singwi, Tosi, Land, and Sjolander, the so-called qSTLS approach. The calculated S(q) exhibits almost perfect agreement with the quantum Monte Carlo simulation data at r{sub s}=1. However, the extent of agreement somewhat diminishes with increasing r{sub s}, particularly for q around 2k{sub F}. Seen in conjunction with the success of qSTLS theory in dealing with correlations in the unpolarized phase, our study suggests that the otherwise celebrated qSTLS theory is not that good in treating the like-spin correlations.
Langevin spin dynamics based on ab initio calculations: numerical schemes and applications.
Rózsa, L; Udvardi, L; Szunyogh, L
2014-05-28
A method is proposed to study the finite-temperature behaviour of small magnetic clusters based on solving the stochastic Landau-Lifshitz-Gilbert equations, where the effective magnetic field is calculated directly during the solution of the dynamical equations from first principles instead of relying on an effective spin Hamiltonian. Different numerical solvers are discussed in the case of a one-dimensional Heisenberg chain with nearest-neighbour interactions. We performed detailed investigations for a monatomic chain of ten Co atoms on top of a Au(0 0 1) surface. We found a spiral-like ground state of the spins due to Dzyaloshinsky-Moriya interactions, while the finite-temperature magnetic behaviour of the system was well described by a nearest-neighbour Heisenberg model including easy-axis anisotropy. PMID:24806308
Multidimensional instability and dynamics of spin avalanches in crystals of nanomagnets.
Jukimenko, O; Dion, C M; Marklund, M; Bychkov, V
2014-11-21
We obtain a fundamental instability of the magnetization-switching fronts in superparamagnetic and ferromagnetic materials such as crystals of nanomagnets, ferromagnetic nanowires, and systems of quantum dots with large spin. We develop the instability theory for both linear and nonlinear stages. By using numerical simulations we investigate the instability properties focusing on spin avalanches in crystals of nanomagnets. The instability distorts spontaneously the fronts and leads to a complex multidimensional front dynamics. We show that the instability has a universal physical nature, with a deep relationship to a wide variety of physical systems, such as the Darrieus-Landau instability of deflagration fronts in combustion, inertial confinement fusion, and thermonuclear supernovae, and the instability of doping fronts in organic semiconductors. PMID:25479521
A Comparison Study of Magnetic Bearing Controllers for a Fully Suspended Dynamic Spin Rig
NASA Technical Reports Server (NTRS)
Choi, Benjamin; Johnson, Dexter; Morrison, Carlos; Mehmed, Oral; Huff, Dennis (Technical Monitor)
2002-01-01
NASA Glenn Research Center (GRC) has developed a fully suspended magnetic bearing system for the Dynamic Spin Rig (DSR) that is used to perform vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust bearing and the associated control system were integrated into the DSR to provide noncontact magnetic suspension and mechanical excitation of the 35 lb vertical rotor with blades to induce turbomachinery blade vibration. A simple proportional-integral-derivative (PID) controller with a special feature for multidirectional radial excitation worked very well to both support and shake the shaft with blades. However, more advanced controllers were developed and successfully tested to determine the optimal controller in terms of sensor and processing noise reduction, smaller rotor orbits, and energy savings for the system. The test results of a variety of controllers we demonstrated up to the rig's maximum allowable speed of 10,000 rpm are shown.
Attitude Dynamics of Spinning Solar Sail “IKAROS” Considering Thruster Plume
NASA Astrophysics Data System (ADS)
Mori, Osamu; Shirasawa, Yoji; Sawada, Hirotaka; Tsuda, Yuichi; Funase, Ryu; Saiki, Takanao; Yamamoto, Takayuki; Motooka, Norizumi; Jifuku, Ryo
In this paper, the attitude dynamics of IKAROS, which is spinning solar sail, are presented. The first mode model of out-of-plane sail deformation (FMM) and multi-particle model (MPM) are introduced to analyze the oscillatory motion of the spinning solar sail. Three oscillation modes are derived from the FMM. They are caused by the nutation motion of the main body, as well as the nutation motion and the out-of-plane oscillation of the sail. The precise attitude motion after sail deployment and reorientation using thrusters is calculated using the MPM considering thruster plume. The IKAROS flight data of the nutation angular velocities of the main body after sail deployment or reorientation using thrusters are nearly equal to the analytical data found using the FMM and MPM.
Autocatalytic spin-crossover transition: Nonlinear dynamics induced by a photothermal instability
NASA Astrophysics Data System (ADS)
Boukheddaden, Kamel; Paez-Espejo, Miguel; Varret, François; Sy, Mouhamadou
2014-06-01
This predictive theoretical contribution demonstrates that spin-crossover (SC) solids, under light in the regime of the thermally induced hysteresis loop, contain all necessary ingredients for observing autocatalytic behaviors. The sustained oscillations of the high-spin (HS) fraction emerge spontaneously as a result of a subtle balance between the nonlinear relaxation of the HS fraction and the photothermal effect caused by a steady light excitation. Here, we perform a detailed analytical study based on linear stability investigations to clarify the conditions of emergence of such phenomena with respect to the system's parameter in SC solids. Very accurate predictions were obtained and confirmed by the numerical investigations. The treatment developed here should generate experimental results on the nonlinear dynamics and self-induced oscillations in SC solids, and furthermore it should open the perspective of future observations of dissipative structures and pattern formation in all kinds of switchable molecular solids.
Dynamical splayed ferromagnetic ground state in the quantum spin ice Yb(2)Sn(2)O(7).
Yaouanc, A; Dalmas de Réotier, P; Bonville, P; Hodges, J A; Glazkov, V; Keller, L; Sikolenko, V; Bartkowiak, M; Amato, A; Baines, C; King, P J C; Gubbens, P C M; Forget, A
2013-03-22
From magnetic, specific heat, (170)Yb Mössbauer effect, neutron diffraction, and muon spin relaxation measurements on polycrystalline Yb(2)Sn(2)O(7), we show that below the first order transition at 0.15 K all of the Yb(3+) ions are long-range magnetically ordered and each has a moment of 1.1 μ(B) which lies at ≃ 10° to a common fourfold cubic axis. The four sublattice moments have four different directions away from this axis and are therefore noncoplanar. We term this arrangement splayed ferromagnetism. This ground state has a dynamical component with a fluctuation rate in the megahertz range. The net ferromagnetic exchange interaction has an anisotropy that favors the local threefold axis. We discuss our results in terms of the phase diagram proposed by Savary and Balents [Phys. Rev. Lett. 108, 037202 (2012)] for a pyrochlore lattice of Kramers 1/2 effective spins. PMID:25166842
Spin dynamics and implications for superconductivity: Some problems with the d-wave scenario
Levin, K.; Zha, Y.; Radtke, R.J.; Si, Q.; Norman, M.R.; Schuttler, H.B.
1993-09-01
We review the spin dynamics of the normal state of the cuprates with special emphasis on neutron data in both the YBa{sub 2}Cu{sub 3}O{sub 7-{delta}} and La{sub 2-x}Sr{sub x}CuO{sub 4} systems. When realistic models of the Fermi surface shapes are incorporated, along with a moderate degree of spin fluctuations, we find good semi-quantiative agreement with experiment for both cuprates. Building on the success of this Fermi-liquid-based scheme, we explore the implications for d-wave pairing from a number of vantage points. We conclude that our present experimental and theoretical understanding is inadequate to confirm or refute the d-wave scenario.
Wylie, Benjamin J; Dzikovski, Boris G.; Pawsey, Shane; Caporini, Marc; Rosay, Melanie; Freed, Jack H.; McDermott, Ann E.
2016-01-01
We demonstrate that dynamic nuclear polarization (DNP) of membrane proteins in lipid bilayers may be achieved using a novel polarizing agent: pairs of spin labels covalently bound to a protein of interest interacting at an intermolecular interaction surface. For gramicidin A, nitroxide tags attached to the N-terminal intermolecular interface region become proximal only when bimolecular channels forms in the membrane. We obtained signal enhancements of 6-fold for the dimeric protein. The enhancement affect was comparable to that of a doubly tagged sample of gramicidin C, with intramolecular spin pairs. This approach could be a powerful and selective means for signal enhancement in membrane proteins, and for recognizing intermolecular interfaces. PMID:25828256
NASA Astrophysics Data System (ADS)
Ertaş, Mehmet
2016-06-01
By using the simplified effective-field theory based on Glauber-type stochastic dynamics, namely the dynamic simplified effective-field theory, the dynamic phase diagrams of a two-dimensional mixed spin-1 and spin-3/2 Blume-Capel model are studied in an oscillating external magnetic field. The dynamic equations are derived for two interpenetrating square lattices. The time variations of average magnetizations and the temperature dependence of the dynamic magnetizations are examined, and the dynamic phase diagrams are presented in the two different planes. The dynamic phase diagrams illustrate several ordered phases, the coexistence phase region and critical points as well as a re-entrant behavior depending on the interaction parameters. Finally, the discussion and comparison of the dynamic phase diagrams are given briefly.
Ripley, Edward B.
2009-11-24
A thermocouple shield for use in radio frequency fields. In some embodiments the shield includes an electrically conductive tube that houses a standard thermocouple having a thermocouple junction. The electrically conductive tube protects the thermocouple from damage by an RF (including microwave) field and mitigates erroneous temperature readings due to the microwave or RF field. The thermocouple may be surrounded by a ceramic sheath to further protect the thermocouple. The ceramic sheath is generally formed from a material that is transparent to the wavelength of the microwave or RF energy. The microwave transparency property precludes heating of the ceramic sheath due to microwave coupling, which could affect the accuracy of temperature measurements. The ceramic sheath material is typically an electrically insulating material. The electrically insulative properties of the ceramic sheath help avert electrical arcing, which could damage the thermocouple junction. The electrically conductive tube is generally disposed around the thermocouple junction and disposed around at least a portion of the ceramic sheath. The concepts of the thermocouple shield may be incorporated into an integrated shielded thermocouple assembly.
DYNAMICAL SPIN SUSCEPTIBILITY IN THE TD-LDA AND QSGW APPROXIMATIONS
SCHILFGAARDE, MARK VAN; KOTANI, TAKAO
2012-10-15
Abstract. This project was aimed at building the transverse dynamical spin susceptibility with the TD-LDA and the recently-developed Quasparticle Self-Consisent Approximations, which determines an optimum quasiparticle picture in a self-consistent manner within the GW approximation. Our main results were published into two papers, (J. Phys. Cond. Matt. 20, 95214 (2008), and Phys. Rev. B83, 060404(R) (2011). In the first paper we present spin wave dispersions for MnO, NiO, and -MnAs based on quasiparticle self-consistent GW approximation (QSGW). For MnO and NiO, QSGW results are in rather good agreement with experiments, in contrast to the LDA and LDA+U descriptions. For -MnAs, we find a collinear ferromagnetic ground state in QSGW, while this phase is unstable in the LDA. In the second, we apply TD-LDA to the CaFeAs2 the first attempt the first ab initio calculation of dynamical susceptibililty in a system with complex electronic structure Magnetic excitations in the striped phase of CaFe2As2 are studied as a function of local moment amplitude. We find a new kind of excitation: sharp resonances of Stoner-like (itinerant) excitations at energies comparable to the ´eel temperature, originating largely from a narrow band of Fe d states near the Fermi level, and coexisting with more conventional (localized) spin waves. Both kinds of excitations can show multiple branches, highlighting the inadequacy of a description based on a localized spin model.
Tracking the charge and spin dynamics of electronic excited states in inorganic complexes
NASA Astrophysics Data System (ADS)
Gaffney, Kelly
2015-03-01
Inorganic complexes have many advantageous properties for solar energy applications, including strong visible absorption and photocatalytic activity. Whether used as a photocatalyst or a photosensitizer, the lifetime of electronic excited states and the earth abundance of the molecular components represent a key property for solar energy applications. These dual needs have undermined the usefulness of many coordination compounds. Isoelectronic iron and ruthenium based complexes represent a clear example. Ru-polypyridal based molecules have been the workhorse of solar energy related research and dye sensitized solar cells for decades, but the replacement of low abundance Ru with Fe leads to million-fold reductions in metal to ligand charge transfer (MLCT) excited state lifetimes. Understanding the origin of this million-fold reduction in lifetime and how to control excited state relaxation in 3d-metal complexes motivates the work I will discuss. We have used the spin sensitivity of hard x-ray fluorescence spectroscopy and the intense femtosecond duration pulses generated by the LCLS x-ray laser to probe the spin dynamics in a series of electronically excited [Fe(CN)6-2N(2,2'-bipyridine)N]2 N - 4 complexes, with N = 1-3. These femtosecond resolution measurements demonstrate that modification of the solvent and ligand environment can lengthen the MLCT excited state lifetime by more than two orders of magnitude. They also verify the role of triplet ligand field excited states in the spin crossover dynamics from singlet to quintet spin configurations. Work supported by the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy.
Field dependent spin dynamics in Dysprosium2Titanium2Oxygen7
NASA Astrophysics Data System (ADS)
Matthews, Maria Jane
We have studied the field dependent magnetic properties of three crystalline directions of the spin ice material Dy2Ti 2O7---the [100], [110], and [111] directions. Comprehensive magnetization and ac susceptibility data were taken in the temperature range 1.8 K < T < 7 K at fields of up to H = 4 T in the frequency range from dc to f = 10 kHz. We found that crystalline anisotropy plays an important role in determining the spin dynamics in this temperature and magnetic field regime, as well as surprising features presenting in the kHz frequency range where the ac measurement is performed faster than the characteristic relaxation time of the system. In particular, the [110] direction showed a distinct region of freezing into the "spin-chain" state and the [111] direction showed a distinct "kagome-ice" region, as well as an unexpected peak at higher frequencies---remnant of the first-order phase transition at lower temperatures. The [110] and [111] crystalline directions were determined to be of enough interest to extend to lower temperature using a much more difficult dilution refrigerator experiment. Two large crystals were provided by groups at Universidad Nacional de La Plata -CONICET, Argentina, and University of Oxford, United Kingdom, respectively, for the additional purpose of probing the spatial variation inside the crystal (as opposed to measuring the whole crystal as is traditionally done in ac susceptibility experiments). Differences between the end and the center of the crystals were observed in an applied field and approaching the higher frequency measurement limit. Additionally, two more projects are presented on the related materials Tb2Ti2O7 and Tb2Ti2-xSn xO7. The former was lead by Sean Giblin and Peter Baker from ISIS, and the latter by Maria Dahlberg from the Pennsylvania State University. A search for the magnetization plateau associated with the quantum spin ice state was the motivation behind the Tb2Ti2O7 study; however, only unusual dynamics in
NASA Astrophysics Data System (ADS)
Lloveras, V.; Badetti, E.; Veciana, J.; Vidal-Gancedo, J.
2016-02-01
In this paper we report the study of the dynamics of a thermally modulated intramolecular spin exchange interaction of a novel diradical nitronyl nitroxide-substituted disulfide in solution and when it is grafted on a gold surface. The structure of this diradical was designed to have flexible chains leading to intramolecular collisions and hence spin exchange interaction, and with an appropriate binding group to be grafted on the gold surface to study its behavior on the surface. In solution, this diradical shows a strong spin exchange interaction between both radicals which is modulated by temperature, but also gold nanoparticles (AuNPs) functionalized with this diradical permit investigation of such a phenomenon in surface-grafted radicals. The spin-labelled AuNP synthesis was optimized to obtain high coverage of spin labels to lead to high spin exchange interaction. The obtained AuNPs were studied by Electron Paramagnetic Resonance (EPR), UV-Vis, and IR spectroscopies, HR-TEM microscopy, Cyclic Voltammetry (CV), Energy Dispersive X-ray analysis (EDX) and Thermogravimetric Analysis (TGA). This inorganic-organic hybrid material also showed dipolar interactions between its radicals which were confirmed by the appearance in the EPR spectra of an |Δms| = 2 transition at half-field. This signal gives direct evidence of the presence of a high-spin state and permitted us to study the nature of the magnetic coupling between the spins which was found to be antiferromagnetic. Self-Assembled Monolayers (SAMs) of these radicals on the Au (111) substrate were also prepared and studied by contact angle, X-Ray Photoelectron Spectroscopy (XPS), Time-of-Flight Secondary Ion Mass Spectrometry (ToF-SIMS), Cyclic Voltammetry and EPR. The magnetic as well as the electrochemical properties of the hybrid surfaces were studied and compared with the properties of this diradical in solution. Analogies between the properties of AuNPs with high coverage of radicals and those of SAM were
NASA Astrophysics Data System (ADS)
Danieli, Ernesto P.; Pastawski, Horacio M.; Álvarez, Gonzalo A.
2005-01-01
We develop the Keldysh formalism for the polarization dynamics of an open spin system. We apply it to the swapping between two qubit states in a model describing an NMR cross-polarization experiment. The environment is a set of interacting spins. For fast fluctuations in the environment, the analytical solution shows effects missed by the secular approximation of the quantum master equation for the density matrix: a frequency decrease depending on the system-environment escape rate and the quantum quadratic short time behavior. Considering full memory of the bath correlations yields a progressive change of the swapping frequency.
Optimal pulse spacing for dynamical decoupling in the presence of a purely dephasing spin bath
Ajoy, Ashok; Alvarez, Gonzalo A.; Suter, Dieter
2011-03-15
Maintaining quantum coherence is a crucial requirement for quantum computation; hence protecting quantum systems against their irreversible corruption due to environmental noise is an important open problem. Dynamical decoupling (DD) is an effective method for reducing decoherence with a low control overhead. It also plays an important role in quantum metrology, where, for instance, it is employed in multiparameter estimation. While a sequence of equidistant control pulses [the Carr-Purcell-Meiboom-Gill (CPMG) sequence] has been ubiquitously used for decoupling, Uhrig recently proposed that a nonequidistant pulse sequence [the Uhrig dynamic decoupling (UDD) sequence] may enhance DD performance, especially for systems where the spectral density of the environment has a sharp frequency cutoff. On the other hand, equidistant sequences outperform UDD for soft cutoffs. The relative advantage provided by UDD for intermediate regimes is not clear. In this paper, we analyze the relative DD performance in this regime experimentally, using solid-state nuclear magnetic resonance. Our system qubits are {sup 13}C nuclear spins and the environment consists of a {sup 1}H nuclear spin bath whose spectral density is close to a normal (Gaussian) distribution. We find that in the presence of such a bath, the CPMG sequence outperforms the UDD sequence. An analogy between dynamical decoupling and interference effects in optics provides an intuitive explanation as to why the CPMG sequence performs better than any nonequidistant DD sequence in the presence of this kind of environmental noise.
Spin Dynamics Simulations of Multiple Echo Spacing Pulse Sequences in Grossly Inhomogeneous Fields
Heidler, R.; Bachman, H. N.; Johansen, Y.
2008-12-05
Pulse sequences with multiple lengths of echo spacings are used in oilfield NMR logging for diffusion-based NMR applications such as rock and fluid characterization. One specific implementation is the so-called diffusion editing sequence comprising two long echo spacings followed by a standard CPMG at a shorter echo spacing. The echoes in the CPMG portion contain signal from both the direct and stimulated echoes.Modern oilfield NMR logging tools are designed for continuous depth logging of earth formations by projecting both the static (B{sub 0}) and dynamic (B{sub 1}) fields into the formation. Both B{sub 0} and B{sub 1} profiles are grossly inhomogeneous which results in non-steady-state behavior in the early echoes. The spin dynamics effects present a challenge for processing the echo amplitudes to measure porosity (amplitude extrapolated to zero time) and attenuations for fluid or pore size characterization.In this work we describe a calculation of the spin dynamics of the diffusion editing sequence with two long echo spacings. The calculation takes into account full B{sub 1} and B{sub 0} field maps, and comparisons will be made for sensors and parameters typical of oilfield logging tools and environments.
Spin dynamics in the negatively charged terbium (III) bis-phthalocyaninato complex.
Branzoli, Francesca; Carretta, Pietro; Filibian, Marta; Zoppellaro, Giorgio; Graf, Michael J; Galan-Mascaros, Jose R; Fuhr, Olaf; Brink, Susan; Ruben, Mario
2009-04-01
The experimental and theoretical study of the electron spin dynamics in the anionic form of a single-ion molecule magnet (SIMM), the bis-phthalocyaninato terbium (III) molecule [Pc(2)Tb](-)[TBA](+), has been addressed by means of solid state (1)H NMR spectroscopy. The magnetic properties of the caged Tb(3+) metal center were investigated in a series of diamagnetically diluted preparations, where the excess of tetrabutylamonium bromide ([TBA]Br)(n) salt was used as diamagnetic matrix complement. We found that a high temperature activated spin dynamics characterizes the systems, which involved phonon-assisted transitions among the crystal field levels in qualitative agreements with literature results. However, the activation barriers in these processes range from 641 cm(-1) for the diamagnetically diluted samples to 584 cm(-1) for those undiluted; thus, they exhibit barriers 2-3 times larger than witnessed in earlier (230 cm(-1)) reports (e.g., Ishikawa, N.; Sugita, M.; Ishikawa, T.; Koshihara, S.; Kaizu, Y. J. Am. Chem. Soc. 2003, 125, 8694-8695). At cryogenic temperatures, fluctuations are driven by tunneling processes between the m = +6 and -6 low-energy levels. We found that the barrier Delta and the tunneling rates change from sample to sample and especially the diamagnetically diluted [Pc(2)Tb](-) molecules appear affected by the sample's magneto/thermal history. These observations emphasize that matrix arrangements around [Pc(2)Tb](-) can appreciably alter the splitting of the crystal field levels, its symmetry, and hence, the spin dynamics. Therefore, understanding how small differences in molecular surroundings (as for instance occurring by depositing on surfaces) can trigger substantial modifications in the SIMM property is of utmost importance for the effective operation of such molecules for single-molecule data storage, for example. PMID:19275145
Instrumentation for solid-state dynamic nuclear polarization with magic angle spinning NMR
NASA Astrophysics Data System (ADS)
Rosay, Melanie; Blank, Monica; Engelke, Frank
2016-03-01
Advances in dynamic nuclear polarization (DNP) instrumentation and methodology have been key factors in the recent growth of solid-state DNP NMR applications. We review the current state of the art of solid-state DNP NMR instrumentation primarily based on available commercial platforms. We start with a general system overview, including options for microwave sources and DNP NMR probes, and then focus on specific developments for DNP at 100 K with magic angle spinning (MAS). Gyrotron microwave sources, passive components to transmit microwaves, the DNP MAS probe, a cooling device for low-temperature MAS, and sample preparation procedures including radicals for DNP are considered.
Understanding Visual Map Formation through Vortex Dynamics of Spin Hamiltonian Models
NASA Astrophysics Data System (ADS)
Cho, Myoung Won; Kim, Seunghwan
2004-01-01
The pattern formation in orientation and ocular dominance columns is one of the most investigated problems in the brain. From a known cortical structure, we build spinlike Hamiltonian models with long-range interactions of the Mexican hat type. These Hamiltonian models allow a coherent interpretation of the diverse phenomena in the visual map formation with the help of relaxation dynamics of spin systems. In particular, we explain various phenomena of self-organization in orientation and ocular dominance map formation including the pinwheel annihilation and its dependency on the columnar wave vector and boundary conditions.
Calibration of the spin-scan ozone imager aboard the dynamics Explorer 1 satellite
NASA Technical Reports Server (NTRS)
Bressette, Walter E.; Keating, Gerald M.; Young, David F.
1987-01-01
The calibration technique, which contains the calibrated backscattered radiance values necessary for performing the calibrations, is presented. The calibration constants for September to October 1981 to determine total columnar ozone from the Spin-Scan Ozone Imager (SOI), which is a part of the auroral imaging instrumentation aboard the Dynamics Explorer 1 Satellite, are provided. The precision of the SOI-derived total columnar ozone is estimated to be better than 2.4 percent. Linear regression analysis was used to calculate correlation coefficients between total columnar ozone obtained from Dobson ground stations and SOI which indicate that the SOI total columnar ozone determination is equally accurate for clear or cloudy weather conditions.
Instrumentation for solid-state dynamic nuclear polarization with magic angle spinning NMR.
Rosay, Melanie; Blank, Monica; Engelke, Frank
2016-03-01
Advances in dynamic nuclear polarization (DNP) instrumentation and methodology have been key factors in the recent growth of solid-state DNP NMR applications. We review the current state of the art of solid-state DNP NMR instrumentation primarily based on available commercial platforms. We start with a general system overview, including options for microwave sources and DNP NMR probes, and then focus on specific developments for DNP at 100K with magic angle spinning (MAS). Gyrotron microwave sources, passive components to transmit microwaves, the DNP MAS probe, a cooling device for low-temperature MAS, and sample preparation procedures including radicals for DNP are considered. PMID:26920834
NASA Astrophysics Data System (ADS)
Filippov, B. N.; Dubovik, M. N.; Korzunin, L. G.
2016-06-01
We study the dynamic properties of asymmetric vortex Bloch walls and classical 1D Néel walls controlled by a spin-polarized current in magnetic films with in-plane anisotropy. It is shown that fairly high velocities of domain walls (up to 100 m/s) can be obtained for the current density in the range j = 106-108 A/cm2. The nonlinear dependence of the wall velocity on the film thickness and the linear dependence of the velocity on the current density and inverse damping parameter are found.
Zhang, Wei; Jungfleisch, Matthias B.; Freimuth, Frank; Jiang, Wanjun; Sklenar, Joseph; Pearson, John E.; Ketterson, John B.; Mokrousov, Yuri; Hoffmann, Axel
2015-10-06
We investigate spin-orbit torques of metallic CuAu-I-type antiferromagnets using spin-torque ferromagnetic resonance tuned by a dc-bias current. The observed spin torques predominantly arise from diffusive transport of spin current generated by the spin Hall effect. We find a growth-orientation dependence of the spin torques by studying epitaxial samples, which may be correlated to the anisotropy of the spin Hall effect. The observed anisotropy is consistent with first-principles calculations on the intrinsic spin Hall effect. Our work suggests large tunable spin-orbit effects in magnetically-ordered materials.
NASA Astrophysics Data System (ADS)
Álvarez, Gonzalo A.; Ajoy, Ashok; Peng, Xinhua; Suter, Dieter
2010-10-01
Avoiding the loss of coherence of quantum mechanical states is an important prerequisite for quantum information processing. Dynamical decoupling (DD) is one of the most effective experimental methods for maintaining coherence, especially when one can access only the qubit system and not its environment (bath). It involves the application of pulses to the system whose net effect is a reversal of the system-environment interaction. In any real system, however, the environment is not static, and therefore the reversal of the system-environment interaction becomes imperfect if the spacing between refocusing pulses becomes comparable to or longer than the correlation time of the environment. The efficiency of the refocusing improves therefore if the spacing between the pulses is reduced. Here, we quantify the efficiency of different DD sequences in preserving different quantum states. We use C13 nuclear spins as qubits and an environment of H1 nuclear spins as the environment, which couples to the qubit via magnetic dipole-dipole couplings. Strong dipole-dipole couplings between the proton spins result in a rapidly fluctuating environment with a correlation time of the order of 100 μs. Our experimental results show that short delays between the pulses yield better performance if they are compared with the bath correlation time. However, as the pulse spacing becomes shorter than the bath correlation time, an optimum is reached. For even shorter delays, the pulse imperfections dominate over the decoherence losses and cause the quantum state to decay.
Kerr rotation studies of single electron spin dynamics in a quantum dot
NASA Astrophysics Data System (ADS)
Mikkelsen, M. H.; Berezovsky, J.; Gywat, O.; Stoltz, N. G.; Coldren, L. A.; Awschalom, D. D.
2007-03-01
Kerr rotation measurements are used to directly and non-destructively probe the dynamics of a single electron spin in a charge-tunable quantum dot. The dot is formed by interface fluctuations of a GaAs quantum well and embedded in a vertical optical cavity. Using Hanle techniques, we perform single electron Kerr rotation measurements at T=10K in order to monitor the depolarization of an optically pumped electron spin within an applied transverse magnetic field. This reveals information about the time averaged transverse spin lifetime, T2^*. At gate voltages for which the charging rate of the dot is relatively low, the results yield a T2^* in agreement with values expected from the hyperfine interaction in these materials. In contrast, at larger charging rates, we find that T2^* is strongly reduced, indicating the importance of additional decoherence mechanisms in that regime. J. Berezovsky, M. H. Mikkelsen, O. Gywat, N. G. Stoltz, L. A. Coldren, and D. D. Awschalom,Science Express, 9 November 2006, (10.1126/science.1133862).
Spin Dynamics and Quantum Tunneling in Fe8 Nanomagnet and in AFM Rings by NMR
Seung-Ho-Baek
2004-12-19
In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs), For this we have selected two different classes of SMMs: a ferrimagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T{sub l}) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs T and H for the first time. For AFM rings, we have shown that 1/T{sub l} probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions.
Absence of Magnetic Order and Persistent Spin Dynamics in Tb2Ge2O7
NASA Astrophysics Data System (ADS)
Hallas, Alannah; Arevalo-Lopez, Angel; Wilson, Murray; Liu, Lian; Attfield, J. Paul; Uemura, Yasutomo; Wiebe, Chris; Luke, Graeme
2015-03-01
The terbium pyrochlores exhibit many unique magnetic properties, which has generated significant interest in this family of frustrated materials. A candidate spin liquid, Tb2Ti2O7 fails to magnetically order, despite strong antiferromagnetic correlations. The application of external pressure has been found to produce partial antiferromagnetic order in Tb2Ti2O7. Recently, we synthesized a new member of this family, Tb2Ge2O7. Due to the large ionic radii decrease from titanium to germanium, Tb2Ge2O7 can be considered a chemical pressure analog of Tb2Ti2O7. However, neutron scattering measurements revealed an absence of magnetic order in Tb2Ge2O7 down to 20 mK and dominant ferromagnetic correlations. Now, we have investigated the low temperature magnetism of Tb2Ge2O7 with muon spin rotation. Our zero field μSR measurements confirm an absence of static order in Tb2Ge2O7. We find a sharp increase in magnetic correlations below 10 K and persistent spin dynamics down to 25 mK. Our longitudinal field μSR measurements on Tb2Ge2O7 at 25 mK are consistent with a system of fluctuating moments, with a fluctuation rate of 11 MHz. This fluctuation rate is nearly temperature independent below 2.5 K.
Magnetic Dynamics of Single-Domain Planar Spin-Transfer Devices
NASA Astrophysics Data System (ADS)
Bazaliy, Ya. B.
2008-03-01
We study spin-transfer devices with dynamic magnets characterized by large easy-plane anisotropy. This situation is standard for planar devices where it arises due to the shape anisotropy. Dominating easy-plane anisotropy keeps the motion of the magnetic moment close to the easy plane, with small out-of-plane deviations. As a result, it is possible to approximately describe magnetization vector by the in-plane angle and derive an effective one dimensional equation for that angle in the absence [1] and in the presence [2] of spin-transfer torques. Effective description maps a spin-transfer device problem onto a problem of an ``effective particle'' moving in external potential with variable friction coefficient. The advantage of such a description is that the motion of the effective particle can be qualitatively understood by applying the usual energy conservation and dissipation arguments. We show how the effective description produces analytic results for current induced precession states [3] and predicts unconventional ``stabilization by repulsion'' of static states [2]. // [1] C. J. Garcia-Cervera, Weinan E, J. Appl. Phys. 90, 370 (2001). [2] Ya. B. Bazaliy, Phys. Rev. B 76, 140402(R) (2007). [3] Ya. B. Bazaliy, arXiv:0705.0508, to be published in Appl. Phys. Lett. (2007).
NASA Technical Reports Server (NTRS)
Creel, T. R., Jr.; Beckwith, I. E. (Inventor)
1982-01-01
An improved test section for a supersonic or hypersonic wind tunnel is disclosed wherein the model tested is shielded from the noise normally radiated by the turbulent tunnel wall boundary layer. A vacuum plenum surrounds spaced rod elements making up the test chamber to extract some of the boundary layer as formed along the rod elements during a test to thereby delay the tendency of the rod boundary layers to become turbulent. Novel rod construction involves bending each rod slightly prior to machining the bent area to provide a flat segment on each rod for connection with the flat entrance fairing. Rods and fairing are secured to provide a test chamber incline on the order of 1 deg outward from the noise shield centerline to produce up to 65% reduction of the root mean square (rms) pressure over previously employed wind tunnel test sections at equivalent Reynolds numbers.
Smith, A W; Bishop, P J; Wells, R P
1985-06-01
The effect of a hockey helmet and face shield on the head and neck during inertial loading was studied. A Hybrid III Anthropometric Test Dummy (ATD) was struck from both the front and rear by a spring-loaded, instrumented striker moving at 2.9 ms-1. Data were collected from a triaxial force transducer mounted at the atlanto-occipital (a-o) junction of the ATD, a load cell in the striker, and by cinematography (250 fps). Angular kinematics of the head and moments of force about the a-o junction were determined along with impact force levels. When compared to a bare-head condition, the addition of a helmet and face shield caused an increase in head angular displacement (20-40%) but did not affect head angular acceleration. Axial and shear forces at the a-o junction did not change appreciably with the addition of a helmet and face shield. A triphasic pattern was evident for the neck moments including a small phase which represented a seating of the headform on the nodding blocks of the uppermost ATD neck segment, and two larger phases of opposite polarity which represented the motion of the head relative to the trunk during the first 350 ms after impact. No substantial differences were apparent between the helmeted and non-helmeted trials. The magnitudes of forces and moments found in the present study were well within tolerance levels reported by others (Melvin, 1979; Cheng et al., 1982). It was concluded that the increase in angular displacement of the head, with the addition of a helmet and face shield, does not place the wearer in a position of increased risk of cervical spine trauma. PMID:4017154
Mentink-Vigier, Frédéric; Paul, Subhradip; Lee, Daniel; Feintuch, Akiva; Hediger, Sabine; Vega, Shimon; De Paëpe, Gaël
2015-09-14
Over the last two decades solid state Nuclear Magnetic Resonance has witnessed a breakthrough in increasing the nuclear polarization, and thus experimental sensitivity, with the advent of Magic Angle Spinning Dynamic Nuclear Polarization (MAS-DNP). To enhance the nuclear polarization of protons, exogenous nitroxide biradicals such as TOTAPOL or AMUPOL are routinely used. Their efficiency is usually assessed as the ratio between the NMR signal intensity in the presence and the absence of microwave irradiation εon/off. While TOTAPOL delivers an enhancement εon/off of about 60 on a model sample, the more recent AMUPOL is more efficient: >200 at 100 K. Such a comparison is valid as long as the signal measured in the absence of microwaves is merely the Boltzmann polarization and is not affected by the spinning of the sample. However, recent MAS-DNP studies at 25 K by Thurber and Tycko (2014) have demonstrated that the presence of nitroxide biradicals combined with sample spinning can lead to a depolarized nuclear state, below the Boltzmann polarization. In this work we demonstrate that TOTAPOL and AMUPOL both lead to observable depolarization at ≈110 K, and that the magnitude of this depolarization is radical dependent. Compared to the static sample, TOTAPOL and AMUPOL lead, respectively, to nuclear polarization losses of up to 20% and 60% at a 10 kHz MAS frequency, while Trityl OX63 does not depolarize at all. This experimental work is analyzed using a theoretical model that explains how the depolarization process works under MAS and gives new insights into the DNP mechanism and into the spin parameters, which are relevant for the efficiency of a biradical. In light of these results, the outstanding performance of AMUPOL must be revised and we propose a new method to assess the polarization gain for future radicals. PMID:26235749
Quantum dynamics of atomic coherence in a spin-1 condensate: Mean-field versus many-body simulation
NASA Astrophysics Data System (ADS)
Plimak, L. I.; Weiß, C.; Walser, R.; Schleich, W. P.
2006-08-01
We analyse and numerically simulate the full many-body quantum dynamics of a spin-1 condensate in the single spatial mode approximation. Initially, the condensate is in a "ferromagnetic" state with all spins aligned along the y axis and the magnetic field pointing along the z axis. In the course of evolution the spinor condensate undergoes a characteristic change of symmetry, which in a real experiment could be a signature of spin-mixing many-body interactions. The results of our simulations are conveniently visualised within the picture of irreducible tensor operators.
Reversal of spin dynamics in an antiferromagnetic F = 1 spinor Bose-Einstein condensate
NASA Astrophysics Data System (ADS)
Schwettmann, Arne; Summy, Gil; Pechkis, Hyewon; Wrubel, Jonathan; Barnett, Ryan; Wilson, Ryan; Tiesinga, Eite; Lett, Paul
2014-05-01
The antiferromagnetic F = 1 sodium spinor Bose-Einstein condensate (BEC) exhibits coherent population oscillations of the magnetic sublevels that are internally driven by spin-exchange collisions. Here, we experimentally demonstrate reversals of the collisional dynamics. The reversals are controlled with microwave pulses. We observe nearly complete reversals even after a significant amount of population oscillation has already occurred. In addition, and somewhat surprisingly, we can generate partial reversals in the cold, non-condensed normal gas. We explain our results with numerical calculations based on the truncated Wigner approximation and an analytical theory based on the Bogoliubov approximation. In the future, this type of microwave control of collisional dynamics will allow us to implement matter-wave analogs of devices known from quantum optics with photons, such as a phase-sensitive matter-wave amplifier.
Sensing Polymer Chain Dynamics through Ring Topology: A Neutron Spin Echo Study.
Gooßen, Sebastian; Krutyeva, Margarita; Sharp, Melissa; Feoktystov, Artem; Allgaier, Jürgen; Pyckhout-Hintzen, Wim; Wischnewski, Andreas; Richter, Dieter
2015-10-01
Using neutron spin echo spectroscopy, we show that the segmental dynamics of polymer rings immersed in linear chains is completely controlled by the host. This transforms rings into ideal probes for studying the entanglement dynamics of the embedding matrix. As a consequence of the unique ring topology, in long chain matrices the entanglement spacing is directly revealed, unaffected by local reptation of the host molecules beyond this distance. In shorter entangled matrices, where in the time frame of the experiment secondary effects such as contour length fluctuations or constraint release could play a role, the ring motion reveals that the contour length fluctuation is weaker than assumed in state-of-the-art rheology and that the constraint release is negligible. We expect that rings, as topological probes, will also grant direct access to molecular aspects of polymer motion which have been inaccessible until now within chains adhering to more complex architectures. PMID:26551826
Application of a system modification technique to dynamic tuning of a spinning rotor blade
NASA Technical Reports Server (NTRS)
Spain, C. V.
1987-01-01
An important consideration in the development of modern helicopters is the vibratory response of the main rotor blade. One way to minimize vibration levels is to ensure that natural frequencies of the spinning main rotor blade are well removed from integer multiples of the rotor speed. A technique for dynamically tuning a finite-element model of a rotor blade to accomplish that end is demonstrated. A brief overview is given of the general purpose finite element system known as Engineering Analysis Language (EAL) which was used in this work. A description of the EAL System Modification (SM) processor is then given along with an explanation of special algorithms developed to be used in conjunction with SM. Finally, this technique is demonstrated by dynamically tuning a model of an advanced composite rotor blade.
The co-evolutionary dynamics of directed network of spin market agents
NASA Astrophysics Data System (ADS)
Horváth, Denis; Kuscsik, Zoltán; Gmitra, Martin
2006-09-01
The spin market model [S. Bornholdt, Int. J. Mod. Phys. C 12 (2001) 667] is generalized by employing co-evolutionary principles, where strategies of the interacting and competitive traders are represented by local and global couplings between the nodes of dynamic directed stochastic network. The co-evolutionary principles are applied in the frame of Bak-Sneppen self-organized dynamics [P. Bak, K. Sneppen, Phys. Rev. Lett. 71 (1993) 4083] that includes the processes of selection and extinction actuated by the local (node) fitness. The local fitness is related to orientation of spin agent with respect to the instant magnetization. The stationary regime is formed due to the interplay of self-organization and adaptivity effects. The fat tailed distributions of log-price returns are identified numerically. The non-trivial model consequence is the evidence of the long time market memory indicated by the power-law range of the autocorrelation function of volatility with exponent smaller than one. The simulations yield network topology with broad-scale node degree distribution characterized by the range of exponents 1.3<γin<3 coinciding with social networks.
Nonlinear dynamics of a strongly driven single spin solid state qubit
NASA Astrophysics Data System (ADS)
Coppersmith, S. N.; Jullien, Thibaut; Scarlino, P.; Kawakami, E.; Ward, D. R.; Savage, D. E.; Lagally, M. G.; Friesen, Mark; Eriksson, M. A.; Vandersypen, L. M. K.
This talk will discuss how dynamical systems theory can yield new insight into some exotic behavior found in experiments on strongly driven quantum spins in silicon/silicon-germanium heterostructures. Spin resonance experiments were performed by using ac voltages to drive an electron wavefunction in a strong magnetic field gradient. Nontrivial dependence of the resonance frequency on applied power, including the observation of multiple resonant frequencies at one power, are shown to be consistent with frequency-dependent attenuation in the high-frequency lines. The method of analysis is very similar to that presented in the course on nonlinear dynamics that Leo Kadanoff developed at the University of Chicago in the early 1990's. This work was supported in part by ARO (W911NF-12-0607). Development and maintenance of the growth facilities used for fabricating samples is supported by DOE (DE-FG02-03ER46028). This research utilized NSF-supported shared facilities at UW-Madison.
Domain wall motion driven by adiabatic spin transfer torque through excitation of nonlinear dynamics
NASA Astrophysics Data System (ADS)
Wang, D.; Dong, Yulan; Yan, Zhou; Wang, Xi-guang; He, Jun; Guo, Guang-hua
2016-05-01
Domain wall dynamics under the joint action of a linearly polarized microwave magnetic field and spin transfer torque was analysed in terms of the domain wall collective coordinates. It was found that a microwave-assisted steady domain wall motion driven by adiabatic spin transfer torque can be adequately described by three domain wall collective coordinates. Analytical expression for the domain wall velocity showed that there are two contributions to the steady domain wall motion. One is derived from the nonlinear oscillation of domain wall width excited by the microwave field, and the other is from the heterodyne process between the width oscillation and the microwave field. The former always propels a domain wall to move in the positive direction, which is defined as the direction of the applied current. The latter contribution to the domain wall velocity can be positive or negative, depending on the polarization of the microwave field. The final domain wall velocity is determined by the competition between those two contributions, which indicates that by simply changing the polarization of the microwave field, the direction of the domain wall motion can be reversed. Our analysis demonstrated that the characteristics of domain wall motion can be tuned by selective excitation of nonlinear domain wall dynamics.
Singularities of the dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field
NASA Astrophysics Data System (ADS)
Carmelo, J. M. P.; Sacramento, P. D.; Machado, J. D. P.; Campbell, D. K.
2015-10-01
We study the longitudinal and transverse spin dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. While the static properties of the model can be studied within a Fermi-liquid like description in terms of pseudoparticles, our derivation of the dynamical properties relies on the introduction of a form of the ‘pseudofermion dynamical theory’ (PDT) of the 1D Hubbard model suitably modified for the spin-only XXX chain and other models with two pseudoparticle Fermi points. Specifically, we derive the exact momentum and spin-density dependences of the exponents {{\\zeta}τ}(k) controlling the singularities for both the longitudinal ≤ft(τ =l\\right) and transverse ≤ft(τ =t\\right) dynamical structure factors for the whole momentum range k\\in ]0,π[ , in the thermodynamic limit. This requires the numerical solution of the integral equations that define the phase shifts in these exponents expressions. We discuss the relation to neutron scattering and suggest new experiments on spin-chain compounds using a carefully oriented crystal to test our predictions.
Singularities of the dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field.
Carmelo, J M P; Sacramento, P D; Machado, J D P; Campbell, D K
2015-10-14
We study the longitudinal and transverse spin dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. While the static properties of the model can be studied within a Fermi-liquid like description in terms of pseudoparticles, our derivation of the dynamical properties relies on the introduction of a form of the 'pseudofermion dynamical theory' (PDT) of the 1D Hubbard model suitably modified for the spin-only XXX chain and other models with two pseudoparticle Fermi points. Specifically, we derive the exact momentum and spin-density dependences of the exponents ζ(τ)(k) controlling the singularities for both the longitudinal (τ = l) and transverse (τ = t) dynamical structure factors for the whole momentum range k ∈ ]0,π[, in the thermodynamic limit. This requires the numerical solution of the integral equations that define the phase shifts in these exponents expressions. We discuss the relation to neutron scattering and suggest new experiments on spin-chain compounds using a carefully oriented crystal to test our predictions. PMID:26403307
NASA Astrophysics Data System (ADS)
Krämer, Sebastian; Ritsch, Helmut
2015-12-01
We numerically study the collective coherent and dissipative dynamics in spin lattices with long range interactions in one, two and three dimensions. For generic geometric configurations with a small spin number, which are fully solvable numerically, we show that a dynamical mean-field approach based upon a spatial factorization of the density operator often gives a surprisingly accurate representation of the collective dynamics. Including all pair correlations at any distance in the spirit of a second order cumulant expansion improves the numerical accuracy by at least one order of magnitude. We then apply this truncated expansion method to simulate large numbers of spins from about ten in the case of the full quantum model, a few thousand, if all pair correlations are included, up to several ten-thousands in the mean-field approximation. We find collective modifications of the spin dynamics in surprisingly large system sizes. In 3D, the mutual interaction strength does not converge to a desired accuracy within the maximum system sizes we can currently implement. Extensive numerical tests help in identifying interaction strengths and geometric configurations where our approximations perform well and allow us to state fairly simple error estimates. By simulating systems of increasing size we show that in one and two dimensions we can include as many spins as needed to capture the properties of infinite size systems with high accuracy. As a practical application our approach is well suited to provide error estimates for atomic clock setups or super radiant lasers using magic wavelength optical lattices.
NASA Astrophysics Data System (ADS)
Montes, H.; Monkenbusch, M.; Willner, L.; Rathgeber, S.; Fetters, L.; Richter, D.
1999-05-01
Diblock copolymers in the melt exhibit order-disorder phase transitions (ODT), which are accompanied by strong concentration fluctuations. These transitions are generally described in terms of the random phase approximation (RPA) of Leibler and Fredrickson, which is able to explain small angle scattering results in the neighborhood of the ODT, in particular around the correlation peak at q*. The RPA theory has been extended to include dynamical phenomena, predicting the short time relaxation of the dynamic structure factor in polymeric multicomponent systems. We report small angle neutron scattering and neutron spin echo experiments on polyethylene-block-polyethylethylene (PE-PEE) and poly(ethylene-propylene)-block-polyethylethylene (PEP-PEE) copolymers with molecular weights of 16.500 and 68.000 g/mol, which explore the structure and dynamics of these block copolymers. Studying melts with different hydrogen/deuterium labeling it was possible to observe experimentally the different relaxation modes of such systems separately. In particular the collective relaxation behavior as well as the single chain motion were accessed. The experimental results were quantitatively compared with the RPA predictions, which were based solely on the dynamical properties of the corresponding homopolymers and the static structure factors. The collective dynamics exhibits an unanticipated fast relaxation mode. This mode is most visible at low wave numbers (q⩾q*) but extends to length scales considerably shorter than the radius of gyration. Furthermore, the dynamical RPA yields expressions for the mobilities of chain segments in the block copolymer melt. These combination rules are at variance with the experimental findings for the single chain dynamics, while they hold for the collective response.
Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7
NASA Astrophysics Data System (ADS)
Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.
2012-09-01
Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.
NASA Technical Reports Server (NTRS)
Bannister, Tommy; Karr, Gerald R.
1987-01-01
Progress on the modeling of the flow field around a wake shield using a recently obtained code based on the Monte Carlo method is discussed. The direct simulation Monte Carlo method is a method for solving the Boltzman Equation using an approximation to the collision integral term. The collision integrand is evaluated for randomly selected values of its arguments and the summation will approach the integral for large enough samples. The collision effects may be modeled for either hard sphere or various power law potentials. The convective side of the Boltzman equation is approximated over a time step using a simple trajectory calculation of molecules as they travel through the domain of interest.
Decoupling a spin qubit from high-frequency Larmor dynamics of a GaAs nuclear spin bath
NASA Astrophysics Data System (ADS)
Malinowski, Filip K.; Martins, Frederico; Nissen, Peter D.; Rudner, Mark S.; Marcus, Charles M.; Kuemmeth, Ferdinand; Barnes, Edwin; Fallahi, Saeed; Gardner, Geoffrey C.; Manfra, Michael J.
We present a technique of decoupling a spin qubit in a GaAs/AlGaAs heterostructure from low- and high-frequency noise arising from hyperfine interaction of electrons with nuclear spins. We use Carr-Purcell-Meiboom-Gill sequences in which we synchronize the repetition rate of π pulses to difference Larmor frequencies of 69Ga, 71Ga and 75As nuclei. This decouples the qubit both from low-frequency noise due to diffusion of nuclear spins and from noise at selected high frequencies, allowing us to apply more than a thousand π pulses in a sequence. We demonstrate a coherence time of a singlet-triplet qubit of 0.87 ms, i.e. five orders of magnitude longer than the inhomogeneous dephasing time intrinsic to GaAs. Support through IARPA-MQCO, Army Research Office, LPS-MPO-CMTC, the Villum Foundation and the Danish National Research Foundation is acknowledged.
Elasto-dynamic analysis of spinning nanodisks via a surface energy-based model
NASA Astrophysics Data System (ADS)
Kiani, Keivan
2016-07-01
Using the surface elasticity theory of Gurtin and Murdoch, in-plane vibrations of annular nanodisks due to their rotary motion are explored. By the imposition of non-classical boundary conditions on the innermost and outermost surfaces and employing Hamilton’s principle, the unknown elasto-dynamic fields of the bulk zone are determined via the finite element method. The roles of both nanodisk geometry and surface effect on the natural frequencies are addressed. Subsequently, forced vibrations of spinning nanodisks with fixed–free and free–free boundary conditions are comprehensively examined. The obtained results show that the maximum dynamic elastic fields grow in a parabolic manner as the steady angular velocity increases. By increasing the outermost radius, the maximum dynamic elastic field is magnified and the influence of the surface effect on the results reduced. This work can be considered as a pivotal step towards optimal design and dynamic analysis of nanorotors with disk-like parts, which are one of the basic building blocks of the upcoming advanced nanotechnologies.
Guo, Y. J.; Gao, Y. J.; Ge, C. N; Guo, Y. Y.; Yan, Z. B.; Liu, J.-M.
2015-05-07
In this work, the dynamics of a diatomic chain is investigated with ↑↑↓↓ spin order in which the dispersion relation characterizes the effect of magnetic interactions on the lattice dynamics. The optical or acoustic mode softening in the center or boundary of the Brillouin zone can be observed, indicating the transitions of ferroelectric state, antiferromagnetic state, or ferroelastic state. The coexistence of the multiferroic orders related to the ↑↑↓↓ spin order represents a type of intrinsic multiferroic with strong ferroelectric order and different microscopic mechanisms.