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Sample records for excited compound nuclei

  1. Stochastic model of angular distributions of fragments originating from the fission of excited compound nuclei

    SciTech Connect

    Hiryanov, R. M.; Karpov, A. V.; Adeev, G. D.

    2008-08-15

    The anisotropy of angular distributions of fission fragments and the average multiplicity of prescission neutrons were calculated within a stochastic approach to fission dynamics on the basis of three-dimensional Langevin equations. This approach was combined with a Monte Carlo algorithm for the degree of freedom K (projection of the total angular momentum I onto the fission axis). The relaxation time {tau}{sub K} in the coordinate K was considered as a free parameter of the model; it was estimated on the basis of a fit to experimental data on the anisotropy of angular distributions. Specifically, the relaxation time {tau}{sub K} was estimated at 2 x 10{sup -21} s for the compound nuclei {sup 224}Th and {sup 225}Pa and at 4 x 10{sup -21} s for the heavier nuclei {sup 248}Cf, {sup 254}Fm, and {sup 264}Rf. The potential energy was calculated on the basis of the liquid-drop model with allowance for finiteness of the range of nuclear forces and for the diffuseness of the nuclear surface. A modified one-body viscosity mechanism featuring a coefficient k{sub s} that takes into account the reduction of the contribution from the wall formula was used to describe collective-energy dissipation. The coefficient k{sub s} was also treated as a free parameter and was estimated at 0.5 on the basis of a fit to experimental data on the average prescission multiplicity of neutrons.

  2. Two-dimensional Langevin modeling of fission dynamics of the excited compound nuclei 188Pt, 227Pa and 251Es

    NASA Astrophysics Data System (ADS)

    Eslamizadeh, H.

    2016-02-01

    A stochastic approach based on one- and two-dimensional Langevin equations is applied to calculate the pre-scission neutron multiplicity, fission probability, anisotropy of fission fragment angular distribution, fission cross section and the evaporation cross section for the compound nuclei 188Pt, 227Pa and 251Es in an intermediate range of excitation energies. The chaos weighted wall and window friction formula are used in the Langevin equations. The elongation parameter, c, is used as the first dimension and projection of the total spin of the compound nucleus onto the symmetry axis, K, considered as the second dimension in Langevin dynamical calculations. A constant dissipation coefficient of K, γK = 0.077(MeV zs)-1/2, is used in two-dimensional calculations to reproduce the above mentioned experimental data. Comparison of the theoretical results of the pre-scission neutron multiplicity, fission probability, fission cross section and the evaporation cross section with the experimental data shows that the results of two-dimensional calculations are in better agreement with the experimental data. Furthermore, it is shown that the two-dimensional Langevin equations together with a dissipation coefficient of K, γK = 0.077(MeV zs)-1/2, can satisfactorily reproduce the anisotropy of fission fragment angular distribution for the heavy compound nucleus 251Es. However, a larger value of γK = 0.250(MeV zs)-1/2 is needed to reproduce the anisotropy of fission fragment angular distribution for the lighter compound nucleus 227Pa.

  3. Measurement of light charged particles in the decay channels of medium-mass excited compound nuclei

    NASA Astrophysics Data System (ADS)

    Valdré, S.; Barlini, S.; Casini, G.; Pasquali, G.; Piantelli, S.; Carboni, S.; Cinausero, M.; Gramegna, F.; Marchi, T.; Baiocco, G.; Bardelli, L.; Benzoni, G.; Bini, M.; Blasi, N.; Bracco, A.; Brambilla, S.; Bruno, M.; Camera, F.; Corsi, A.; Crespi, F.; D'Agostino, M.; Degerlier, M.; Kravchuk, V. L.; Leoni, S.; Million, B.; Montanari, D.; Morelli, L.; Nannini, A.; Nicolini, R.; Poggi, G.; Vannini, G.; Wieland, O.; Bednarczyk, P.; Ciemała, M.; Dudek, J.; Fornal, B.; Kmiecik, M.; Maj, A.; Matejska-Minda, M.; Mazurek, K.; Męczyński, W. M.; Myalski, S.; Styczeń, J.; Ziębliński, M.

    2014-03-01

    The 48Ti on 40Ca reactions have been studied at 300 and 600 MeV focusing on the fusion-evaporation (FE) and fusion-fission (FF) exit channels. Energy spectra and multiplicities of the emitted light charged particles have been compared to Monte Carlo simulations based on the statistical model. Indeed, in this mass region (A ~ 100) models predict that shape transitions can occur at high spin values and relatively scarce data exist in the literature about coincidence measurements between evaporation residues and light charged particles. Signals of shape transitions can be found in the variations of the lineshape of high energy gamma rays emitted from the de-excitation of GDR states gated on different region of angular momenta. For this purpose it is important to keep under control the FE and FF processes, to regulate the statistical model parameters and to control the onset of possible pre-equilibrium emissions from 300 to 600 MeV bombarding energy.

  4. Complex fragment emission from hot compound nuclei

    SciTech Connect

    Moretto, L.G.

    1986-03-01

    The experimental evidence for compound nucleus emission of complex fragments at low energies is used to interpret the emission of the same fragments at higher energies. The resulting experimental picture is that of highly excited compound nuclei formed in incomplete fusion processes which decay statistically. In particular, complex fragments appear to be produced mostly through compound nucleus decay. In the appendix a geometric-kinematic theory for incomplete fusion and the associated momentum transfer is outlined. 10 refs., 19 figs.

  5. Fission barriers of compound superheavy nuclei.

    PubMed

    Pei, J C; Nazarewicz, W; Sheikh, J A; Kerman, A K

    2009-05-15

    The dependence of fission barriers on the excitation energy of the compound nucleus impacts the survival probability of superheavy nuclei synthesized in heavy-ion fusion reactions. In this work, we investigate the isentropic fission barriers by means of the self-consistent nuclear density functional theory. The relationship between isothermal and isentropic descriptions is demonstrated. Calculations have been carried out for 264Fm, 272Ds, ;{278}112, ;{292}114, and ;{312}124. For nuclei around ;{278}112 produced in "cold-fusion" reactions, we predict a more rapid decrease of fission barriers with excitation energy as compared to the nuclei around ;{292}114 synthesized in "hot-fusion" experiments. This is explained in terms of the difference between the ground-state and saddle-point temperatures. The effect of the particle gas is found to be negligible in the range of temperatures studied. PMID:19518948

  6. Systematic Study of Fission Barriers of Excited Superheavy Nuclei

    SciTech Connect

    Sheikh, J. A.; Nazarewicz, Witold; Pei, J. C.

    2009-01-01

    A systematic study of fission-barrier dependence on excitation energy has been performed using the self-consistent finite-temperature Hartree-Fock+BCS (FT-HF+BCS) formalism with the SkM* Skyrme energy density functional. The calculations have been carried out for even-even superheavy nuclei with Z ranging between 110 and 124. For an accurate description of fission pathways, the effects of triaxial and reflection asymmetric degrees of freedom have been fully incorporated. Our survey demonstrates that the dependence of isentropic fission barriers on excitation energy changes rapidly with particle number, pointing to the importance of shell effects even at large excitation energies characteristic of compound nuclei. The fastest decrease of fission barriers with excitation energy is predicted for deformed nuclei around N = 164 and spherical nuclei around N = 184 that are strongly stabilized by ground-state shell effects. For nuclei ^{240}Pu and ^{256}Fm, which exhibit asymmetric spontaneous fission, our calculations predict a transition to symmetric fission at high excitation energies due to the thermal quenching of static reflection asymmetric deformations.

  7. M1 excitation scheme in deformed nuclei

    NASA Astrophysics Data System (ADS)

    Otsuka, Takaharu; Morrison, Iain

    1991-10-01

    We present the M1 excitation scheme in even-even deformed nuclei from the sum-rule viewpoint based on the Nilsson+BCS approach. The sum-rule states are introduced for the Scissors, spin and spin-flip modes. The functional form of the B(M1) sum rule of the Scissors mode is obtained, and its actual value is shown to be 4˜6(μN2). The spin excitation B(M1) is 10˜15(μN2) including the spin-flip transitions. The total B(M1) is 15˜20(μN2). The effect of the SD and SDG pair truncation is studied to test IBM-2 for M1 excitations. The SDG truncation reproduces very well the calculation without truncation. The SD truncation reproduces the orbital excitation, whereas yields some deviations for the spin excitation.

  8. Fission Barriers of Compound Superheavy Nuclei

    SciTech Connect

    Pei, Junchen; Nazarewicz, Witold; Sheikh, J. A.; Kerman, A. K.

    2009-01-01

    The dependence of fission barriers on the excitation energy of the compound nucleus impacts the survival probability of superheavy nuclei synthesized in heavy-ion fusion reactions. We study the temperature-dependent fission barriers by means of the self-consistent nuclear density functional theory. The equivalence of isothermal and isentropic descriptions is demonstrated. The effect of the particle gas is found to be negligible in the range of temperatures studied. Calculations have been carried out for ^{264}Fm, ^{272}Ds, ^{278}112, ^{292}114, and ^{312}124. For nuclei around ^{278}112 produced in "cold fusion" reactions, we predict a more rapid decrease of fission barriers with temperature as compared to the nuclei around ^{292}114 synthesized in "hot fusion" experiments. This is explained in terms of the difference between the ground-state and fission-barrier temperatures. Our calculations are consistent with the long survival probabilities of the superheavy elements produced in Dubna with the ^{48}Ca beam.

  9. Fusion excitation functions involving transitional nuclei

    SciTech Connect

    Rehm, K.E.; Jiang, C.L.; Esbensen, H.

    1995-08-01

    Measurements of fusion excitation functions involving transitional nuclei {sup 78}Kr and {sup 100}Mo showed a different behavior at low energies, if compared to measurements with {sup 86}Kr and {sup 92}Mo. This points to a possible influence of nuclear structure on the fusion process. One way to characterize the structure of vibrational nuclei is via their restoring force parameters C{sub 2} which can be calculated from the energy of the lowest 2{sup +} state and the corresponding B(E2) value. A survey of the even-even nuclei between A = 28-150 shows strong variations in C{sub 2} values spanning two orders of magnitude. The lowest values for C{sub 2} are observed for {sup 78}Kr, {sup 104}Ru and {sup 124}Xe followed by {sup 74,76}Ge, {sup 74,76}Se, {sup 100}Mo and {sup 110}Pd. In order to learn more about the influence of {open_quotes}softness{close_quotes} on the sub-barrier fusion enhancement, we measured cross sections for evaporation residue production for the systems {sup 78}Kr + {sup 104}Ru and {sup 78}Kr + {sup 76}Ge with the gas-filled magnet technique. For both systems, fusion excitation functions involving the closed neutron shell nucleus {sup 86}Kr were measured previously. The data are presently being analyzed.

  10. Fission Barriers and Neutron Gas in Compound Superheavy Nuclei

    SciTech Connect

    Pei, Junchen; Nazarewicz, W.; Sheikh, J. A.; Kerman, A. K.

    2010-01-01

    Fission and neutron emission are the principal cooling mechanisms of the compound superheavy nuclei. In the framework of the Finite-Temperature Hartree-Fock-Bogoliubov method, the fission barriers and neutron gas have been studied in the excited superheavy systems. Very different energy dependence of fission barriers has been found for ^{278}112 and ^{292}114. On the other hand, the energy dependence of thermal neutron gas has been found to be almost identical for both systems.

  11. Shells Evolution and Core Excitations in Semi-Magic Nuclei

    NASA Astrophysics Data System (ADS)

    Nowacki, F.

    2007-04-01

    Recent advances in Large Shell Model calculations allow now to treat extended valence spaces and more complete descriptions of (semi-)magic nuclei can be achieved with inclusion of core excitations. The interplay between shell evolution and core excitations in semi-magic nuclei will be illustrated for tin isotopic chains in the framework of Large Shell Model calculations. pn and nn monopole relative influence will be traced back on Effective Single Particle Energies and B(E2)'s.

  12. The Photoresponse of Atomic Nuclei: Collective Excitations and Photodissociation

    NASA Astrophysics Data System (ADS)

    Zilges, A.; Babilon, M.; van den Berg, A. M.; Galaviz, D.; Hasper, J.; Harakeh, M. N.; Lindenberg, K.; Müller, S.; Ramspeck, K.; Savran, D.; Sonnabend, K.; Volz, S.; Wörtche, H. J.; Zarza, M.

    2006-04-01

    The dipole strength distribution of atomic nuclei below the particle threshold has been investigated systematically in photon scattering experiments. A concentration of electric dipole strength around 7 MeV exhausting up to 1% of the Energy Weighted Sum Rule has been observed in all nuclei studied so far. The detailed structure of these excitations and the connection to a resonance-like concentration of E1 strength above the threshold found in neutron-rich radioactive nuclei is still not understood. The latest strength measurements and new experiments with hadrons to study the isospin character of the excitations are discussed.

  13. Collective excitation spectra of transitional even nuclei

    SciTech Connect

    Quentin, P. Paris-11 Univ., 91 - Orsay . Centre de Spectrometrie Nucleaire et de Spectrometrie de Masse); Deloncle, I.; Libert, J. . Centre de Spectrometrie Nucleaire et de Spectrometrie de Masse); Sauvage, J. . Inst. de Physique Nucleaire)

    1990-11-06

    This talk is dealing with the nuclear low energy collective motion as described in the context of microscopic versions of the Bohr Hamiltonian. Two different ways of building microscopically Bohr collective Hamiltonians will be sketched; one within the framework of the Generator Coordinate Method, the other using the Adiabatic Time-Dependent Hartree-Fock-Boholyubov approximation. A sample of recent results will be presented which pertains to the description of transitional even nuclei and to the newly revisited phenomenon of superdeformation at low spin.

  14. Exotic modes of excitation in proton rich nuclei

    SciTech Connect

    Paar, N.

    2011-11-30

    The framework of relativistic energy density functional has been applied in description of excitation phenomena in nuclei close to the proton drip line. In particular, low-lying dipole excitations have been studied using relativistic quasiparticle random phase approximation, based on effective Lagrangians with density dependent meson nucleon couplings. In the isovector dipole channel, the occurrence of pronounced low-lying dipole peaks is predicted, corresponding to the proton pygmy dipole resonance. Since this exotic mode still awaits its experimental confirmation, systematic calculations have been conducted within a pool of neutron deficient nuclei, in order to identify the best possible candidates for measurements.

  15. Coulomb excitation studies of shape coexistence in atomic nuclei

    NASA Astrophysics Data System (ADS)

    Görgen, Andreas; Korten, Wolfram

    2016-02-01

    Low-energy Coulomb excitation provides a well-understood means of exciting atomic nuclei and allows measuring electromagnetic moments that can be directly related to the nuclear shape. The availability of radioactive ion beams (RIBs) at energies near the Coulomb barrier has made it possible to study shape coexistence in a variety of short-lived exotic nuclei. This review presents a short overview of the methods related to multi-step Coulomb excitation experiments, followed by a discussion of several examples. The focus is on two mass regions where recent Coulomb excitation experiments have contributed to the quantitative understanding of shape coexistence: nuclei with mass A≈ 70 near the N = Z line and nuclei with A ≈ 100 near neutron number N = 60. Experimental results are summarized and their significance for understanding shape coexistence is discussed. Experimental observables such as quadrupole moments and electromagnetic transition strengths represent furthermore important benchmarks for advancing theoretical nuclear structure models. With several new RIB facilities planned and under construction, Coulomb excitation will remain to be an important tool to extend the studies of nuclear shapes toward more exotic systems, and to obtain a more comprehensive and quantitative understanding of shape coexistence.

  16. Isomeric States and Collective Excitations of Heaviest Nuclei

    NASA Astrophysics Data System (ADS)

    Adamian, G. G.; Antonenko, N. V.; Jolos, R. V.; Kuzmina, A. N.; Malov, L. A.; Shirikova, N. Yu.; Sushkov, A. V.

    2013-03-01

    The isotopic dependence of two-quasiparticle isomeric states in Fm and No is treated. An α-decay chain through the isomeric states of super-heavy nuclei is demonstrated. The excitation energies and the structure of the low lying states with Kπ = 0‒ 1‒ 2‒ are calculated with the quasiparticle phonon model.

  17. Core excitation effects in the breakup of halo nuclei

    SciTech Connect

    Moro, A. M.; Diego, R. de; Lay, J. A.; Crespo, R.; Johnson, R. C.; Arias, J. M.; Gomez-Camacho, J.

    2012-10-20

    The role of core excitation in the structure and dynamics of two-body halo nuclei is investigated. We present calculations for the resonant breakup of {sup 11}Be on protons at an incident energy of 63.7 MeV/nucleon, where core excitation effects were shown to be important. To describe the reaction, we use a recently developed extension of the DWBA formalism which incorporates these core excitation effects within the no-recoil approximation. The validity of the no-recoil approximation is also examined by comparing with DWBA calculations which take into account core recoil. In addition, calculations with two different continuum representations are presented and compared.

  18. Bulk Properties of Nuclear Matter From Excitations of Nuclei

    SciTech Connect

    Shlomo, Shalom

    2007-10-26

    We consider the predictive power of Hartree-Fock (HF) approximation in determining properties of finite nuclei and thereby in extracting bulk properties of infinite nuclear matter (NM) by extrapolation. In particular, we review the current status of determining the value of NM incompressibility coefficient K, considering the most sensitive method of analyzing the recent accurate experimental data on excitation strengths of compression modes of nuclei within microscopic relativistic and non-relativistic theoretical models. We discuss the consequences of common violations of self-consistency in HF based random-phase-approximation calculations of strength functions and present results of highly accurate calculations of centroid energies and excitation cross sections of giant resonances. Explanations (resolutions) of long standing discrepancies in the value of K are presented.

  19. The liquid to vapor phase transition in excited nuclei

    SciTech Connect

    Elliott, J.B.; Moretto, L.G.; Phair, L.; Wozniak, G.J.; Beaulieu, L.; Breuer, H.; Korteling, R.G.; Kwiatkowski, K.; Lefort, T.; Pienkowski, L.; Ruangma, A.; Viola, V.E.; Yennello, S.J.

    2001-05-08

    For many years it has been speculated that excited nuclei would undergo a liquid to vapor phase transition. For even longer, it has been known that clusterization in a vapor carries direct information on the liquid-vapor equilibrium according to Fisher's droplet model. Now the thermal component of the 8 GeV/c pion + 197 Au multifragmentation data of the ISiS Collaboration is shown to follow the scaling predicted by Fisher's model, thus providing the strongest evidence yet of the liquid to vapor phase transition.

  20. Calculation of nuclear reaction cross sections on excited nuclei with the coupled-channels method

    SciTech Connect

    Kawano, T.; Talou, P.; Lynn, J. E.; Chadwick, M. B.; Madland, D. G.

    2009-08-15

    We calculate nuclear cross sections on excited nuclei in the fast neutron energy range. We partition the whole process into two contributions: the direct reaction part and the compound nuclear reactions. A coupled-channels method is used for calculating the direct transition of the nucleus from the initial excited state, which is a member of the ground-state rotational band, to the final ground and excited low-lying levels. This process is strongly affected by the channel coupling. The compound nuclear reactions on the excited state are calculated with the statistical Hauser-Feshbach model, with the transmission coefficients obtained from the coupled-channels calculation. The calculations are performed for a strongly deformed nucleus {sup 169}Tm, and selected cross sections for the ground and first excited states are compared. The calculation is also made for actinides to investigate possible modification to the fission cross section when the target is excited. It is shown that both the level coupling for the entrance channel, and the different target spin, change the fission cross section.

  1. Recent results on giant dipole resonance decays in highly excited nuclei

    SciTech Connect

    Snover, K.A.

    1991-12-31

    Some recent results on Giant Dipole Resonance (GDR) decays in highly excited, equilibrated nuclei, are discussed based primarily on work done at Seattle. Four sections address the following topics: oblate shapes of rotating, highly excited Zr--Mo nuclei; adiabatic versus `motionally narrowed` GDR decay; large spin-driven deformations observed in hot medium-mass nuclei; and search for entrance channel effects in GDR decay following {sup 58}Ni {plus} {sup 92}Zr fusion. 22 refs.

  2. Recent results on giant dipole resonance decays in highly excited nuclei

    SciTech Connect

    Snover, K.A.

    1991-01-01

    Some recent results on Giant Dipole Resonance (GDR) decays in highly excited, equilibrated nuclei, are discussed based primarily on work done at Seattle. Four sections address the following topics: oblate shapes of rotating, highly excited Zr--Mo nuclei; adiabatic versus motionally narrowed' GDR decay; large spin-driven deformations observed in hot medium-mass nuclei; and search for entrance channel effects in GDR decay following [sup 58]Ni [plus] [sup 92]Zr fusion. 22 refs.

  3. Influence of Neutron Enrichment on Disintegration Modes of Compound Nuclei

    SciTech Connect

    Bonnet, E.; Gomez Del Campo, Jorge; Galindo-Uribarri, Alfredo {nmn}; Shapira, Dan

    2008-11-01

    Cross sections, kinetic energy and angular distributions of fragments with charge 6 {le} Z {le} 28 emitted in {sup 78,82}Kr+{sup 40}C at 5.5 MeV/A reactions were measured at the GANIL facility using the INDRA apparatus. This experiment aims to investigate the influence of the neutron enrichment on the decay mechanism of excited nuclei. Data are discussed in comparison with predictions of transition state and Hauser-Feshbach models.

  4. Compound nucleus formation in reactions between massive nuclei: Fusion barrier

    SciTech Connect

    Antonenko, N.V.; Cherepanov, E.A.; Nasirov, A.K.; Permjakov, V.P.; Volkov, V.V.

    1995-05-01

    The evaporation residue cross sections {sigma}{sub ER} in reactions between massive nuclei have been analyzed within different models of complete fusion. The calculations in the framework of the optical model, the surface friction model, and the macroscopic dynamic model can give the results which are by few orders of magnitude different from experimental data. This takes place due to neglect of the competition between complete fusion and quasifission. A possible mechanism of compound nucleus formation in heavy-ion-induced reactions has been suggested. The analysis of the complete fusion of nuclei on the basis of dinuclear system approach has allowed one to reveal an important feature of the fusion process of massive nuclei, that is, the appearance of the fusion barrier during dinuclear system evolution to a compound nucleus. As a result, the competition between complete fusion and quasifission arises and strongly reduces the cross section of the compound nucleus formation. A model is proposed for calculation of this competition in a massive symmetric dinuclear system. This model is applied for collision energies above the Coulomb barrier. The {sigma}{sub ER} values calculated in the framework of dinuclear system approach seem to be close to the experimental data. For illustration the reactions {sup 100}Mo+{sup 100}Mo, {sup 110}Pd+{sup 110}Pd, and {sup 124}Sn+{sup 96}Zr have been considered.

  5. Observation of low- and high-energy Gamow-Teller phonon excitations in nuclei.

    PubMed

    Fujita, Y; Fujita, H; Adachi, T; Bai, C L; Algora, A; Berg, G P A; von Brentano, P; Colò, G; Csatlós, M; Deaven, J M; Estevez-Aguado, E; Fransen, C; De Frenne, D; Fujita, K; Ganioğlu, E; Guess, C J; Gulyás, J; Hatanaka, K; Hirota, K; Honma, M; Ishikawa, D; Jacobs, E; Krasznahorkay, A; Matsubara, H; Matsuyanagi, K; Meharchand, R; Molina, F; Muto, K; Nakanishi, K; Negret, A; Okamura, H; Ong, H J; Otsuka, T; Pietralla, N; Perdikakis, G; Popescu, L; Rubio, B; Sagawa, H; Sarriguren, P; Scholl, C; Shimbara, Y; Shimizu, Y; Susoy, G; Suzuki, T; Tameshige, Y; Tamii, A; Thies, J H; Uchida, M; Wakasa, T; Yosoi, M; Zegers, R G T; Zell, K O; Zenihiro, J

    2014-03-21

    Gamow-Teller (GT) transitions in atomic nuclei are sensitive to both nuclear shell structure and effective residual interactions. The nuclear GT excitations were studied for the mass number A = 42, 46, 50, and 54 "f-shell" nuclei in ((3)He, t) charge-exchange reactions. In the (42)Ca → (42)Sc reaction, most of the GT strength is concentrated in the lowest excited state at 0.6 MeV, suggesting the existence of a low-energy GT phonon excitation. As A increases, a high-energy GT phonon excitation develops in the 6-11 MeV region. In the (54)Fe → (54)Co reaction, the high-energy GT phonon excitation mainly carries the GT strength. The existence of these two GT phonon excitations are attributed to the 2 fermionic degrees of freedom in nuclei. PMID:24702355

  6. On the excitation energy of deep-hole states in medium-heavy-mass spherical nuclei

    NASA Astrophysics Data System (ADS)

    Kolomiytsev, G. V.; Igashov, S. Yu.; Urin, M. H.

    2016-01-01

    Within the particle-hole dispersive optical model it is shown that the spreading effect determines a significant part of the anomalously large excitation energy of deep-hole states in the 90Zr and 208Pb parent nuclei.

  7. Quartet excitations and cluster spectra in light nuclei

    NASA Astrophysics Data System (ADS)

    Cseh, J.; Riczu, G.

    2016-06-01

    The relation of quarteting and clustering in atomic nuclei is discussed based on symmetry-considerations. This connection enables us to predict a complete high-energy cluster spectrum from the description of the low-energy quartet part. As an example the 28Si nucleus is considered, including its well-established ground-state region, the recently proposed superdeformed band, and the high-lying molecular resonances.

  8. Low lying electric dipole excitations in nuclei of the rare earth region

    SciTech Connect

    von Brentano, P.; Zilges, A.; Herzberg, R.D. . Inst. fuer Kernphysik); Zamfir, N.V. ); Kneissl, U.; Heil, R.D.; Pitz, H.H. . Inst. fuer Strahlenphysik); Wesselborg, C. . Inst. fuer Kernphysik)

    1992-01-01

    From many experiments with low energy photon scattering on deformed rare earth nuclei we have obtained detailed information about the distribution of electric dipole strength below 4 MeV. Apart from some weaker transitions between 2 and 4 MeV we observed one, and sometimes two, very strong El-groundstate transitions around 1.5 MeV in all examined nuclei. They arise from the de-excitation of the bandheads of the (J[sup [pi

  9. Probing clustering in excited alpha-conjugate nuclei

    NASA Astrophysics Data System (ADS)

    Borderie, B.; Raduta, Ad. R.; Ademard, G.; Rivet, M. F.; De Filippo, E.; Geraci, E.; Le Neindre, N.; Alba, R.; Amorini, F.; Cardella, G.; Chatterjee, M.; Guinet, D.; Lautesse, P.; La Guidara, E.; Lanzalone, G.; Lanzano, G.; Lombardo, I.; Lopez, O.; Maiolino, C.; Pagano, A.; Papa, M.; Pirrone, S.; Politi, G.; Porto, F.; Rizzo, F.; Russotto, P.; Wieleczko, J. P.

    2016-04-01

    The fragmentation of quasi-projectiles from the nuclear reaction 40Ca+12C at 25 MeV per nucleon bombarding energy was used to produce α-emission sources. From a careful selection of these sources provided by a complete detection and from comparisons with models of sequential and simultaneous decays, evidence in favor of α-particle clustering from excited 16O, 20Ne and 24Mg is reported.

  10. Properties of high-energy isoscalar monopole excitations in medium-heavy mass spherical nuclei

    SciTech Connect

    Gorelik, M. L. Shlomo, Sh. Tulupov, B. A. Urin, M. H.

    2015-07-15

    The recently developed particle-hole dispersive optical model is applied to describe properties of high-energy isoscalar monopole excitations in medium-heavy mass spherical nuclei. In particular, the double transition density averaged over the energy of the isoscalar monopole excitations is considered for {sup 208}Pb in a wide energy interval, which includes the isoscalar giant monopole resonance and its overtone. The energy-averaged strength functions of these resonances are also analyzed.

  11. Exotic modes of excitation in deformed neutron-rich nuclei

    SciTech Connect

    Yoshida, Kenichi

    2011-05-06

    Low-lying dipole excitation mode in neutron-rich Mg isotopes close to the drip line is investigated in the framework of the Hartree-Fock-Bogoliubov and the quasiparticle random-phase approximation employing the Skyrme and the pairing energy-density functionals. It is found that the low-lying dipole-strength distribution splits into the K{sup {pi}} = 0{sup -} and 1{sup -} components due to the nuclear deformation. The low-lying dipole strength increases as the neutron drip-line is approached.

  12. TOPICAL REVIEW: Shapes and collectivity of exotic nuclei via low-energy Coulomb excitation

    NASA Astrophysics Data System (ADS)

    Görgen, Andreas

    2010-10-01

    The way in which an atomic nucleus responds to excitations, whether by promoting individual nucleons into higher shells or by collective rotation or vibration, reveals many details of the underlying nuclear structure. The response of the nucleus is closely related to its macroscopic shape. Low-energy Coulomb excitation provides a well-understood means of exciting atomic nuclei, allowing the measurement of static and dynamic electromagnetic moments as a probe of the nuclear wavefunctions. Owing to the availability of radioactive heavy-ion beams with energies near the Coulomb barrier, it is now possible to study the shape and collectivity of short-lived nuclei far from β stability (the so-called exotic nuclei), providing a particularly stringent test of modern theoretical nuclear structure models. This review gives an introduction to the experimental techniques related to low-energy Coulomb excitation with radioactive ion beams and summarizes the results that were obtained over the last 10 years for a wide variety of exotic nuclei at various laboratories employing the isotope separation on-line technique.

  13. Emission of charged particles from excited compound nuclei

    SciTech Connect

    Kalandarov, Sh. A.; Adamian, G. G.; Antonenko, N. V.; Scheid, W.

    2010-10-15

    The process of complex fragment emission is studied within the dinuclear system model. Cross sections of complex fragment emission are calculated and compared with experimental data for the reactions {sup 3}He+{sup nat}Ag, {sup 78,86}Kr+{sup 12}C, and {sup 63}Cu+{sup 12}C. The mass distributions of the products of these reactions, isotopic distributions for the {sup 3}He+{sup nat}Ag and {sup 78}Kr+{sup 12}C reactions, and average total kinetic energies of the products of the {sup 78}Kr+{sup 12}C reaction are predicted.

  14. Coulomb excitation of exotic nuclei at the R3B-LAND setup

    NASA Astrophysics Data System (ADS)

    Rossi, D. M.; Adrich, P.; Aksouh, F.; Alvarez-Pol, H.; Aumann, T.; Benlliure, J.; Böhmer, M.; Boretzky, K.; Casarejos, E.; Chartier, M.; Chatillon, A.; Cortina-Gil, D.; Datta Pramanik, U.; Emling, H.; Ershova, O.; Fernandez-Dominguez, B.; Geissel, H.; Gorska, M.; Heil, M.; Johansson, H.; Junghans, A.; Kiselev, O.; Klimkiewicz, A.; Kratz, J. V.; Kurz, N.; Labiche, M.; Le Bleis, T.; Lemmon, R.; Litvinov, Yu A.; Mahata, K.; Maierbeck, P.; Movsesyan, A.; Nilsson, T.; Nociforo, C.; Palit, R.; Paschalis, S.; Plag, R.; Reifarth, R.; Simon, H.; Sümmerer, K.; Wagner, A.; Walus, W.; Weick, H.; Winkler, M.

    2013-03-01

    Exotic Ni isotopes have been measured at the R3B-LAND setup at GSI in Darmstadt, using Coulomb excitation in inverse kinematics at beam energies around 500 MeV/u. As the experimental setup allows kinematically complete measurements, the excitation energy was reconstructed using the invariant mass method. The GDR and additional low-lying strength have been observed in 68Ni, the latter exhausting 4.1(1.9)% of the E1 energy-weighted sum rule. Also, the branching ratio for the non-statistical decay of the excited 68Ni nuclei was measured and amounts to 24(4)%.

  15. Halo or skin in the excited states of some light mirror nuclei

    NASA Astrophysics Data System (ADS)

    Chen, J. G.; Cai, X. Z.; Shen, W. Q.; Ma, Y. G.; Ren, Z. Z.; Zhang, H. Y.; Jiang, W. Z.; Zhong, C.; Wei, Y. B.; Guo, W.; Zhou, X. F.; Wang, K.; Ma, G. L.

    2005-01-01

    The properties of three pairs of mirror nuclei 13N- 13C, 15N- 15O and 21Na- 21Ne (these mirror nuclei are all made of a good inert core plus an unpaired valence nucleon) are investigated by using the nonlinear relativistic mean-field (RMF) theory. It is found that the calculated binding energies with two different parameter sets are very close to the experimental ones for both the ground states and the excited states except for the large deformed nuclei. The calculations show that the 2 s1/2 excited states of 15N and of 21Na are both weakly bound with a proton halo and a proton skin (or a pigmy proton skin), respectively. In addition, the 1 d5/2 excited state of 13C and the 2 s1/2 excited state of 15O are also weakly bound with a neutron skin, respectively. The ratio of the valence nucleon radius to matter radius is deduced and it can be regarded as an additional criterion for the existence of exotic structure. The unbound 2 s1/2 and 1 d5/2 excited states of 13N are also discussed.

  16. Compound-Nucleus Formation Following Direct Interactions to Highly-Excited Final States

    SciTech Connect

    Dietrich, F S

    2008-02-05

    When direct reactions populate highly excited, unbound configurations in the residual nucleus, the nucleus may further evolve into a compound nucleus. Alternatively, the residual system may decay by emitting particles into the continuum. Understanding the relative weights of these two processes as a function of the angular momentum and parity deposited in the nucleus is important for the surrogate-reaction technique. A particularly interesting case is compound-nucleus formation via the (d, p) reaction, which may be a useful tool for forming compound nuclei off the valley of stability in inverse-kinematics experiments. We present here a study of the compound formation probability for a closely-related direct reaction, direct-semidirect radiative neutron capture.

  17. Excited states of deformable odd {sup 157,159}Tb nuclei: Nonconservation of the angular momentum of external nucleon

    SciTech Connect

    Sharipov, Sh.; Ermamatov, M. J.

    2009-01-15

    The previously developed rotationally single-particle and vibrational model of the triaxial deformable odd nuclei is extended to the case where the total angular momentum of an external nucleon is not conserved. The calculated ratios of the excitation energies of the {sup 157,159}Tb nuclei are compared with the existing experimental data. The ratios of E2-transition probabilities and those of quadrupole moments of the above nuclei are calculated using parameters determined from the spectra of these nuclei.

  18. Open-shell nuclei and excited states from multireference normal-ordered Hamiltonians

    NASA Astrophysics Data System (ADS)

    Gebrerufael, Eskendr; Calci, Angelo; Roth, Robert

    2016-03-01

    We discuss the approximate inclusion of three-nucleon (3 N ) interactions into ab initio nuclear structure calculations using a multireference formulation of normal ordering and Wick's theorem. Following the successful application of single-reference normal ordering for the study of ground states of closed-shell nuclei, e.g., in coupled-cluster theory, multireference normal ordering opens a path to open-shell nuclei and excited states. Based on different multideterminantal reference states we benchmark the truncation of the normal-ordered Hamiltonian at the two-body level in no-core shell-model calculations for p -shell nuclei, including 6Li,12C, and 10B. We find that this multireference normal-ordered two-body approximation is able to capture the effects of the 3 N interaction with sufficient accuracy, both for ground-state and excitation energies, at the computational cost of a two-body Hamiltonian. It is robust with respect to the choice of reference states and has a multitude of applications in ab initio nuclear structure calculations of open-shell nuclei and their excitations as well as in nuclear reaction studies.

  19. Study of viscosity on the fission dynamics of the excited nuclei 228U produced in 19F + 209Bi reactions

    NASA Astrophysics Data System (ADS)

    Eslamizadeh, H.

    2015-06-01

    A two-dimensional (2D) dynamical model based on Langevin equations was applied to study the fission dynamics of the compound nuclei 228U produced in 19F + 209Bi reactions at intermediate excitation energies. The distance between the centers of masses of the future fission fragments was used as the first dimension and the projection of the total spin of the compound nucleus onto the symmetry axis, K, was considered as the second dimension in Langevin dynamical calculations. The magnitude of post-saddle friction strength was inferred by fitting measured data on the average pre-scission neutron multiplicity for 228U. It was shown that the results of calculations are in good agreement with the experimental data by using values of the post-saddle friction equal to 6-8 × 1021s-1.

  20. Equilibrium deformations and excitation energies of single-quasiproton band heads of rare-earth nuclei

    NASA Astrophysics Data System (ADS)

    Nazarewicz, W.; Riley, M. A.; Garrett, J. D.

    1990-05-01

    Noncollective single-proton states in odd- Z (Eu, Tb, Ho, Tm, Lu, Ta, Ir and Au) rare-earth nuclei have been calculated using the shell correction method with an average Woods-Saxon potential and a monopole pairing residual interaction. Calculated equilibrium deformations of the lowest single-proton states are presented, and calculated band head excitation energies are compared with experimental proton band heads for odd- Z rare-earth nuclei. Good agreement is found between the experimental and calculated band heads. We find that strong polarisation effects due to the odd proton explain many of the systematic trends of known band heads. Different deformation driving forces of the odd-proton orbitals can also partly explain deviations seen in high-spin data. Shape co-existence effects in Ir and Au isotopes are discussed. In addition, equilibrium deformations of even-even rare-earth nuclei are computed and compared with experimental values.

  1. Quantum Monte Carlo calculations of excited states in A=6-8 nuclei

    SciTech Connect

    Pieper, Steven C.; Wiringa, R.B.; Carlson, J.

    2004-11-01

    A variational Monte Carlo method is used to generate sets of orthogonal trial functions, {psi}{sub T}(J{sup {pi}};T), for given quantum numbers in various light p-shell nuclei. These {psi}{sub T} are then used as input to Green's function Monte Carlo (GFMC) calculations of first, second, and higher excited (J{sup {pi}};T) states. Realistic two- and three-nucleon interactions are used. We find that if the physical excited state is reasonably narrow, the GFMC energy converges to a stable result. With the combined Argonne v{sub 18} two-nucleon and Illinois-2 three-nucleon interactions, the results for many second and higher states in A=6-8 nuclei are close to the experimental values.

  2. Excitation of Δ and N* resonances in isobaric charge-exchange reactions of heavy nuclei

    NASA Astrophysics Data System (ADS)

    Vidaña, I.; Benlliure, J.; Geissel, H.; Lenske, H.; Scheidenberger, C.; Vargas, J.

    2016-01-01

    We present a model for the study of the excitation of Δ(1232) and N*(1440) resonances in isobaric charge-exchange (AZ, A(Z ± 1)) reactions of heavy nuclei. Quasi-elastic and inelastic elementary processes contributing to the double differential cross sections of the reactions are described in terms of the exchange of virtual pions. The inelastic channel includes processes where the resonances are excited both in the target and in the projectile nucleus. We present results for reactions of 112Sn and 124Sn on different targets. Our results confirm that the position of the Δ peak is insensitive to targets with mass number A ≥ 12, and show that the origin of the Δ peak shift towards low excitation energies, with respect to its position in reactions with a proton target, can be easily explained in terms of the superposition of the different excitation mechanisms contributing to the reaction.

  3. KEWPIE2: A cascade code for the study of dynamical decay of excited nuclei

    NASA Astrophysics Data System (ADS)

    Lü, Hongliang; Marchix, Anthony; Abe, Yasuhisa; Boilley, David

    2016-03-01

    KEWPIE-a cascade code devoted to investigating the dynamical decay of excited nuclei, specially designed for treating very low probability events related to the synthesis of super-heavy nuclei formed in fusion-evaporation reactions-has been improved and rewritten in C++ programming language to become KEWPIE2. The current version of the code comprises various nuclear models concerning the light-particle emission, fission process and statistical properties of excited nuclei. General features of the code, such as the numerical scheme and the main physical ingredients, are described in detail. Some typical calculations having been performed in the present paper clearly show that theoretical predictions are generally in accordance with experimental data. Furthermore, since the values of some input parameters cannot be determined neither theoretically nor experimentally, a sensibility analysis is presented. To this end, we systematically investigate the effects of using different parameter values and reaction models on the final results. As expected, in the case of heavy nuclei, the fission process has the most crucial role to play in theoretical predictions. This work would be essential for numerical modeling of fusion-evaporation reactions.

  4. Branching ratios of {alpha} decay to excited states of even-even nuclei

    SciTech Connect

    Wang, Y. Z.; Zhang, H. F.; Dong, J. M.; Royer, G.

    2009-01-15

    Branching ratios of {alpha} decay to members of the ground state rotational band and excited 0{sup +} states of even-even nuclei are calculated in the framework of the generalized liquid drop model (GLDM) by taking into account the angular momentum of the {alpha} particle and the excitation probability of the daughter nucleus. The calculation covers isotopic chains from Hg to Fm in the mass regions 180=}224. The calculated branching ratios of the {alpha} transitions are in good agreement with the experimental data and some useful predictions are provided for future experiments.

  5. Role of compound nuclei in intermediate-energy heavy-ion reactions

    SciTech Connect

    Moretto, L.G.; Wozniak, G.J.

    1988-05-01

    Hot compound nuclei are frequently produced in intermediate-energy reactions through a variety of processes. Their decay is shown to be an important and at times dominant source of complex fragments, high energy-gamma rays, and even pions.

  6. Excitation energies of double isobar-analog states in heavy nuclei

    SciTech Connect

    Poplavskii, I. V.

    1988-12-01

    Several new relationships are established for isomultiplets on the basis of a theory in which the Coulomb coupling constant (CCC) is allowed to be complex. In particular, the following rule is formulated: the energies for fission or decay of members of an isomultiplet into a charged cluster and members of the corresponding daughter isomultiplet are equidistant. This relationship is well satisfied for isomultiplets with /ital A/less than or equal to60. By extrapolating the rule for fission and decay energies to the region of heavy nuclei, the excitation energies /ital E//sub /ital x// of double isobar-analog states (DIASs) are found for the nuclei /sup 197,199/Hg, /sup 205/Pb, /sup 205 - -209/Po, /sup 209/At, and /sup 238/Pu. A comparison of the computed energies /ital E//sub /ital x// with the experimentally measured values for /sup 208/Po attest to the reliability and good accuracy of the method proposed here when used to determine the excitation energies of DIASs in heavy nuclei.

  7. Fragmentation of mixed-symmetry excitations in stable even-even tellurium nuclei

    SciTech Connect

    Hicks, S. F.; Vanhoy, J. R.; Yates, S. W.

    2008-11-15

    The lowest six excited 2{sup +} levels of the even-even {sup 122-130}Te nuclei have been investigated using {gamma}-ray spectroscopy following inelastic neutron scattering. These levels have been identified and their decay properties have been characterized from {gamma}-ray excitation functions and {gamma}-ray angular distributions; additionally, lifetimes of these levels have been deduced using the Doppler-shift attenuation method. Electromagnetic transition rates and E2/M1 multipole mixing ratios from the 2{sub x}{sup +}[x=2-6]{yields}2{sub 1}{sup +} transitions have been examined to identify the lowest mixed-symmetry states in these nuclei. In each nucleus, the mixed-symmetry strength appears to be fragmented between more than one level. The summed M1 strength from the 2{sub x}{sup +}[x=2-6] states to the 2{sub 1}{sup +} level agrees rather well with neutron-proton interacting boson model predictions in the U(5) or O(6) limits for these Te nuclei.

  8. Emission of charged particles from excited compound nucleus

    SciTech Connect

    Kalandarov, Sh. A.; Adamian, G. G.; Antonenko, N. V.

    2010-11-24

    The formation and decay of excited compound nucleus are studied within the dinuclear system model[1]. The cross sections of complex fragment emission are calculated and compared with experimental data for the reactions {sup 3}He+{sup 108}Ag, {sup 78,82}Kr+{sup 12}C. Angular momentum dependence of cluster emission in {sup 78}Kr+{sup 12}C and {sup 40}Ca+{sup 78}Kr reactions is demonstrated.

  9. Systematics of the First 2{sup +} Excitation in Spherical Nuclei with Skyrme-QRPA

    SciTech Connect

    Terasaki, J.

    2009-05-07

    We use the Quasiparticle Random Phase Approximation (QRPA) and the Skyrme interactions SLy4 and SkM* to systematically calculate energies and transition strengths for the lowest 2{sup +} state in spherical even-even nuclei. The SkM* functional, applied to 178 spherical nuclei between Z = 10 and 90, produces excitation energies that are on average 11% higher than experimental values, with residuals that fluctuate about the average by -35%+55%. The predictions of SkM* and SLy4 have significant differences, in part because of differences in the calculated ground state deformations; SkM* performs better in both the average and dispersion of energies. Comparing the QRPA results with those of generator-coordinate-method (GCM) calculations, we find that the QRPA reproduces trends near closed shells better than the GCM, and overpredicts the energies less severely in general.

  10. Interplay between collective and single particle excitations around neutron-rich doubly-magic nuclei

    NASA Astrophysics Data System (ADS)

    Leoni, S.

    2016-05-01

    The excitation spectra of nuclei with one or two particles outside a doubly-magic core are expected to be dominated, at low energy, by the couplings between phonon excitations of the core and valence particles. A survey of the experimental situation is given for some nuclei lying in close proximity of neutron-rich doubly-magic systems, such as 47,49Ca, 133Sb and 210Bi. Data are obtained with various types of reactions (multinucleon transfer with heavy ions, cold neutron capture and neutron induced fission of 235U and 241Pu targets), with the employment of complex detection systems based on HPGe arrays. A comparison with theoretical calculations is also presented, in terms of large shell model calculations and of a phenomenological particle-phonon model. In the case of 133Sb, a new microscopic "hybrid" model is introduced: it is based on the coupling between core excitations (both collective and non-collective) of the doubly-magic core and the valence nucleon, using the Skyrme effective interaction in a consistent way.

  11. Excitation of atomic nuclei in hot plasma through resonance inverse electron bridge

    NASA Astrophysics Data System (ADS)

    Tkalya, E. V.; Akhrameev, E. V.; Arutyunyan, R. V.; Bol'shov, L. A.; Kondratenko, P. S.

    2014-09-01

    A process of nucleus excitation by photons under the mechanism of the inverse electron bridge (IEB) is examined provided the energies of atomic and nuclear transitions coincide. It is shown that in this case, the excitation of nuclei with EL[ML] transition with the energy ωN≲10keV is strengthened relative to the process of photoabsorption by nucleus by a factor of 1/(ωNr0)2(L +2) [e4/(ωNr0)2(L+2)], where r0 is a typical size of domain in the ion shell for accumulation of electronic integrals. In the Rb84 nuclei the IEB cross section for the 3.4 keV M1 transition 6-(463.59 keV) ↔5-(463.59keV ) can exceed even a photoexcitation cross section for the 3.4keVE1 transition with the reduced probability in the Weisskopf model BW .u.(E1)=1. This result can be important for understanding the mechanisms of atomic nucleus excitation in hot plasma. In particular, the considered process is capable to provide the existence of so called gamma luminescence wave or a nuclear isomer "burning" wave—an analog of self-maintaining process of triggered depopulation of nuclear isomer.

  12. Delta excitations in heavy nuclei induced by (3He,t) and (p,n) reactions

    NASA Astrophysics Data System (ADS)

    Esbensen, H.; Lee, T.-S. H.

    1985-12-01

    Delta excitations in heavy nuclei, induced by charge exchange reactions, are studied using the surface response model. The residual pion-exchange interaction and the self-energy of the delta in a nuclear medium is included in the random-phase-approximation response. The peak position observed in (3He,t) reactions can be explained by the self-energy of the delta extracted from pion-nucleus scattering, and the magnitude of the cross section is consistent with Glauber theory. The comparison to (p,n) data is reasonable; contributions from neutron decay of the delta, which are left out in the calculations, constitute a substantial experimental background.

  13. Isospin excitation and electromagnetic transition properties of nuclei 88,90Mo

    NASA Astrophysics Data System (ADS)

    Zhang, J. F.; Li, X. W.; Li, Y. S.

    2016-07-01

    The band structure and electromagnetic transition properties of the low-lying states of 88,90Mo isotopes were investigated using the interacting boson model with isospin (IBM-3). The lowest isospin excitation states with T = 2 for 88Mo and T = 3 for 90Mo were identified, and compared with available data. The E2, M1 matrix elements and quadrupole moments for the low-lying states were investigated. Results showed that the lowest mixed-symmetry states were 23+ for 90Mo and 24+ for 88Mo. The excitation energy of the 11+ states in nuclei 88,90Mo were also determined. Good agreement was achieved between calculated results using the model and measured data.

  14. Low lying electric dipole excitations in nuclei of the rare earth region

    SciTech Connect

    von Brentano, P.; Zilges, A.; Herzberg, R.D.; Zamfir, N.V.; Kneissl, U.; Heil, R.D.; Pitz, H.H.; Wesselborg, C.

    1992-10-01

    From many experiments with low energy photon scattering on deformed rare earth nuclei we have obtained detailed information about the distribution of electric dipole strength below 4 MeV. Apart from some weaker transitions between 2 and 4 MeV we observed one, and sometimes two, very strong El-groundstate transitions around 1.5 MeV in all examined nuclei. They arise from the de-excitation of the bandheads of the (J{sup {pi}},K)=(l{sup {minus}},0) and (J{sup {pi}},K)=(l{sup {minus}},1) octupole vibrational bands. It is shown that the decay branching ratios and the absolute transition strengths of these states can be reproduced rather well with an improved T(El)-operator in the sdf-Interacting Boson Model. Another class of octupole states has been investigated in the region of the semimagic nucleus {sup 142}Nd. Here a quintuplet of collective excitations around 3.5 MeV is expected due to the coupling of the 3{minus}-octupole vibration with the 2+-quadrupole vibration. We performed photon scattering experiments on the odd A neighboring nucleus {sup 141}Pr and found first evidence for the existence of 3{sup {minus}}{circle_times}2+{circle_times}particle-states.

  15. Contribution of excited states to stellar weak-interaction rates in odd-A nuclei

    NASA Astrophysics Data System (ADS)

    Sarriguren, P.

    2016-05-01

    Weak-interaction rates, including β decay and electron capture, are studied in several odd-A nuclei in the p f -shell region at various densities and temperatures of astrophysical interest. Special attention is paid to the relative contribution to these rates of thermally populated excited states in the decaying nucleus. The nuclear structure involved in the weak processes is studied within a quasiparticle random-phase approximation with residual interactions in both particle-hole and particle-particle channels on top of a deformed Skyrme Hartree-Fock mean field with pairing correlations. In the range of densities and temperatures considered, it is found that the total rates do not differ much from the rates of the ground state fully populated. In any case, the changes are not larger than the uncertainties due to the nuclear-model dependence of the rates.

  16. A statistical model for simulating the emission of light particles from excited nuclei

    NASA Astrophysics Data System (ADS)

    Sannikov, A. V.; Savitskaya, E. N.

    2016-05-01

    The algorithms and basic equations of a novel evaporation model that have been implemented in the program package EVAP15 are detailed. The level density of an excited nucleus is described by the composite Gilbert-Cameron formula with parameter values as suggested by the IAEA working group RIPL-3. Special attention is paid to the cross sections of inverse reactions and, in particular, to those for the interactions of low-energy neutrons with nuclei and for crossing of the Coulomb barrier by low-energy charged particles. The model predictions are compared with a large volume of experimental data on the spectra of particles emitted in the reactions ( n, xn), ( n, xp), and ( n, xα) induced by neutrons with energy near 14 MeV and on the four spectra for the reaction ( p, xp) induced by 62-MeV protons.

  17. Study of a soft quadrupole excitation in the nucleus [sup 11]Li: A phase space model of neutron halo nuclei

    SciTech Connect

    Yanhuang, C.; Smerzi, A.; Di Toro, M. , P.O. Box 8730, Beijing, 100080 Institute of Nuclear Research, Academia Sinica, P.O. Box 800204, Shanghai 201800 INFN-Laboratorio Nazionale del Sud and Dipartimento di Fisica, 57, Corso Italia, 95129 Catania )

    1994-12-01

    Quadrupole excitations in the nucleus [sup 11]Li have been studied in a semiclassical framework using the nuclear Vlasov equation solved with the test particle method. A soft mode of quadrupole excitation located around 2 MeV is found. The strength (in percentage of the energy-weighted sum rule) exhausted in such a soft quadrupole excitation region is very sensitive to the extension of the neutron halo in the nucleus [sup 11]Li. The results are discussed in comparison with other recent calculations. The use of the collective response to tune phase-space models of neutron excess nuclei to be used in collision dynamics is finally stressed.

  18. Low-lying dipole excitations in vibrational nuclei: The Cd isotopic chain studied in photon scattering experiments

    SciTech Connect

    Kohstall, C.; Belic, D.; Kneissl, U.; Nord, A.; Pitz, H.H.; Scheck, M.; Stedile, F.; Brentano, P. von; Fransen, C.; Gade, A.; Herzberg, R.-D.; Jolie, J.; Linnemann, A.; Pietralla, N.; Werner, V.; Yates, S.W.

    2005-09-01

    High-resolution nuclear resonance fluorescence experiments (NRF) were performed on {sup 110,111,112,114,116}Cd at the bremsstrahlung facility of the 4.3-MV Dynamitron accelerator in Stuttgart to study the low-lying dipole strength distributions in these vibrational nuclei. Numerous excited states, most of them previously unknown, were observed in the excitation energy range up to 4 MeV. Detailed spectroscopic information has been obtained on excitation energies, spins, decay widths, decay branchings, and transition probabilities. For states in the even-even isotopes {sup 110,112,114,116}Cd, parities could be assigned from linear polarization measurements. Together with our previous results for {sup 108,112,113,114}Cd from NRF studies without polarization measurements, systematics was established for the dipole strength distributions of the stable nuclei within the Cd isotopic chain. The results are discussed with respect to the systematics of E1 two-phonon excitations and mixed-symmetry states in even-even nuclei near the Z=50 shell closure and the fragmentation of these excitation modes in the odd-mass Cd isotopes.

  19. The Fe II Emission in Active Galactic Nuclei: Excitation Mechanisms and Location of the Emitting Region

    NASA Astrophysics Data System (ADS)

    Marinello, M.; Rodríguez-Ardila, A.; Garcia-Rissmann, A.; Sigut, T. A. A.; Pradhan, A. K.

    2016-04-01

    We present a study of Fe ii emission in the near-infrared region (NIR) for 25 active galactic nuclei (AGNs) to obtain information about the excitation mechanisms that power it and the location where it is formed. We employ an NIR Fe ii template derived in the literature and find that it successfully reproduces the observed Fe ii spectrum. The Fe ii bump at 9200 Å detected in all objects studied confirms that Lyα fluorescence is always present in AGNs. The correlation found between the flux of the 9200 Å bump, the 1 μm lines, and the optical Fe ii implies that Lyα fluorescence plays an important role in Fe ii production. We determined that at least 18% of the optical Fe ii is due to this process, while collisional excitation dominates the production of the observed Fe ii. The line profiles of Fe ii λ10502, O i λ11287, Ca ii λ8664, and Paβ were compared to gather information about the most likely location where they are emitted. We found that Fe ii, O i and Ca ii have similar widths and are, on average, 30% narrower than Paβ. Assuming that the clouds emitting the lines are virialized, we show that the Fe ii is emitted in a region twice as far from the central source than Paβ. The distance, though, strongly varies: from 8.5 light-days for NGC 4051 to 198.2 light-days for Mrk 509. Our results reinforce the importance of the Fe ii in the NIR to constrain critical parameters that drive its physics and the underlying AGN kinematics, as well as more accurate models aimed at reproducing this complex emission.

  20. X-ray excited Auger transitions of Pu compounds

    SciTech Connect

    Nelson, Art J. Grant, William K.; Stanford, Jeff A.; Siekhaus, Wigbert J.; Allen, Patrick G.; McLean, William

    2015-05-15

    X-ray excited Pu core–valence–valence and core–core–valence Auger line-shapes were used in combination with the Pu 4f photoelectron peaks to characterize differences in the oxidation state and local electronic structure for Pu compounds. The evolution of the Pu 4f core-level chemical shift as a function of sputtering depth profiling and hydrogen exposure at ambient temperature was quantified. The combination of the core–valence–valence Auger peak energies with the associated chemical shift of the Pu 4f photoelectron line defines the Auger parameter and results in a reliable method for definitively determining oxidation states independent of binding energy calibration. Results show that PuO{sub 2}, Pu{sub 2}O{sub 3}, PuH{sub 2.7}, and Pu have definitive Auger line-shapes. These data were used to produce a chemical state (Wagner) plot for select plutonium oxides. This Wagner plot allowed us to distinguish between the trivalent hydride and the trivalent oxide, which cannot be differentiated by the Pu 4f binding energy alone.

  1. The Structure of Excited 0{sup +} States in Nuclei and the Effect of the {gamma} Degree of Freedom

    SciTech Connect

    Sharpey-Schafer, J. F.

    2011-10-28

    The physics of intrinsic states, within the pairing gap of deformed nuclei with N{approx}90 neutrons, is discussed in the light of the recent realization that the first excited 0{sub 2}{sup +} states in these nuclei are not {beta}-vibrations but four quasi-neutron states. The properties of {gamma}-vibration K{sup {pi}} = 2{sup +} bands is discussed. A method of measuring two proton transfer in high resolution using the ({sup 3}He,n) reaction is proposed.

  2. Do nuclei go pear-shaped? Coulomb excitation of 220Rn and 224Ra at REX-ISOLDE (CERN)

    NASA Astrophysics Data System (ADS)

    Scheck, M.; Gaffney, L. P.; Butler, P. A.; Hayes, A. B.; Wenander, F.; Albers, M.; Bastin, B.; Bauer, C.; Blazhev, A.; Boenig, S.; Bree, N.; Cederkall, J.; Chupp, T.; Cline, D.; Cocolios, T. E.; Davinson, T.; De Witte, H.; Diriken, J.; Grahn, T.; Herzan, A.; Huyse, M.; Jenkins, D. G.; Joss, D. T.; Kesteloot, N.; Konki, J.; Kowalczyk, M.; Kroell, Th.; Kwan, E.; Lutter, R.; Moschner, K.; Napiorkowski, P.; Pakarinen, J.; Pfeiffer, M.; Radeck, D.; Reiter, P.; Reynders, K.; Rigby, S. V.; Robledo, L. M.; Rudigier, M.; Sambi, S.; Seidlitz, M.; Siebeck, B.; Stora, T.; Thoele, P.; Van Duppen, P.; Vermeulen, M. J.; von Schmid, M.; Voulot, D.; Warr, N.; Wimmer, K.; Wrzosek-Lipska, K.; Wu, C. Y.; Zielinska, M.

    2015-05-01

    The IS475 collaboration conducted Coulomb-excitation experiments with post-accelerated radioactive 220Rn and 224Ra beams at the REX-ISOLDE facility. The beam particles (Ebeam: 2.83 MeV/u) were Coulomb excited using 60Ni, 114Cd, and 120Sn scattering targets. De-excitation γ-rays were detected employing the Miniball array and scattered particles were detected in a silicon detector. Exploiting the Coulomb-excitation code GOSIA for each nucleus several matrix elements could be obtained from the measured γ-ray yields. The extracted ‹3-||E3||0+› matrix element allows for the conclusion that, while 220Rn represents an octupole vibrational system, 224Ra has already substantial octupole correlations in its ground state. This finding has implications for the search of CP-violating Schiff moments in the atomic systems of the adjacent odd-mass nuclei.

  3. Giant dipole resonance built on hot rotating nuclei produced during evaporation of light particles from the 88Mo compound nucleus

    NASA Astrophysics Data System (ADS)

    Ciemała, M.; Kmiecik, M.; Maj, A.; Mazurek, K.; Bracco, A.; Kravchuk, V. L.; Casini, G.; Barlini, S.; Baiocco, G.; Bardelli, L.; Bednarczyk, P.; Benzoni, G.; Bini, M.; Blasi, N.; Brambilla, S.; Bruno, M.; Camera, F.; Carboni, S.; Cinausero, M.; Chbihi, A.; Chiari, M.; Corsi, A.; Crespi, F. C. L.; D'Agostino, M.; Degerlier, M.; Fornal, B.; Giaz, A.; Gramegna, F.; Krzysiek, M.; Leoni, S.; Marchi, T.; Matejska-Minda, M.; Mazumdar, I.; Meczyński, W.; Million, B.; Montanari, D.; Morelli, L.; Myalski, S.; Nannini, A.; Nicolini, R.; Pasquali, G.; Piantelli, S.; Prete, G.; Roberts, O. J.; Schmitt, Ch.; Styczeń, J.; Szpak, B.; Valdré, S.; Wasilewska, B.; Wieland, O.; Wieleczko, J. P.; Ziebliński, M.; Dudek, J.; Dinh Dang, N.

    2015-05-01

    High-energy giant dipole resonance (GDR) γ rays were measured following the decay of the hot, rotating compound nucleus of 88Mo, produced at excitation energies of 124 and 261 MeV. The reaction 48Ti + 40Ca at 300 and 600 MeV bombarding energies has been used. The data were analyzed using the statistical model Monte Carlo code gemini++. It allowed extracting the giant dipole resonance parameters by fitting the high-energy γ -ray spectra. The extracted GDR widths were compared with the available data at lower excitation energy and with theoretical predictions based on (i) The Lublin-Strasbourg drop macroscopic model, supplemented with thermal shape fluctuations analysis, and (ii) The phonon damping model. The theoretical predictions were convoluted with the population matrices of evaporated nuclei from the statistical model gemini++. Also a comparison with the results of a phenomenological expression based on the existing systematics, mainly for lower temperature data, is presented and discussed. A possible onset of a saturation of the GDR width was observed around T =3 MeV.

  4. Formation of Heavy Compound Nuclei, Their Survival and Correlation with Longtime-Scale Fission

    SciTech Connect

    Karamian, S. A.; Yakushev, A.-B.

    2007-05-22

    Fusion of two massive nuclei with formation of super-heavy compound nucleus (CN) is driven by the potential energy gradient, as follows from the analysis of nuclear reaction cross-sections. The conservative energy of the system is deduced in simple approximation using regularized nuclear mass and interaction barrier values. Different reaction for the synthesis of Zc (110-118) nuclei are compared and the favourable conditions are found for fusion of the stable (W-Pt) isotopes with radioactive fission fragment projectiles, like 94Kr or 100Sr. Thus, the cold fusion method can be extended for a synthesis of elements with Z > 113. Survival of the evaporation residue is defined by the neutron-to-fission probability ratio and by the successful emission of gammas at final step of the reaction. Numerical estimates are presented. Fixation of evaporation residue products must correlate with longtime-scale fission and available experimental results are discussed.

  5. Energy Approach to Resonance states of Compound Superheavy Nucleus and EPPP in Heavy Nuclei Collisions

    SciTech Connect

    Glushkov, Alexander V.

    2005-10-26

    A consistent unified energy approach (operator perturbation theory) is used for numerical calculations of the electron-positron pair production cross-section in heavy nuclei collisions. Resonance phenomena in the nuclear subsystem lead to the structurization of the positron spectrum produced. The positron spectrum narrow peaks are treated as resonance states of the compound superheavy nucleus. Calculation results for the differential cross-sections of the U-U collision energies E1 (E1=162.0keV- third s-resonance; E1=247.6keV- the fourth s-resonance) are presented.

  6. Coulomb Excitation and One-Neutron Transfer Studies of Stable and Radioactive Nuclei at HRIBF-ORNL

    SciTech Connect

    Allmond, James M

    2015-01-01

    Several stable and radioactive nuclei ranging from $A=58$ to 208 were recently studied in inverse kinematics by Coulomb excitation and heavy-ion induced one-neutron transfer at the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory. These studies used a CsI-HPGe detector array to detect scattered charged particles and emitted $\\gamma$ rays from the in-beam reactions. A Bragg-curve detector was used to measure the energy loss of the various beams through the targets and to measure the radioactive beam compositions. Stable nickel, strontium, zirconium, molybdenum, tin, tellurium, and lead isotopes and neutron-rich radioactive tin and tellurium isotopes were among the nuclei recently studied. Coulomb excitation was used to measure the electromagnetic moments of the first excited states and heavy-ion induced one-neutron transfer was used to measure the absolute cross sections and lifetimes of the excited single-particle states. A sample of these results are presented here with an emphasis on the tin isotopes. In particular, a survey of the Bragg-curve measurements, Doppler corrections, and inconclusive $i_{13/2}$ candidate in $^{133}$\\textrm{Sn} are presented.

  7. Interplay of collective and single-particle properties of excited states of deformable odd nuclei {sup 155}Eu and {sup 161}Tm

    SciTech Connect

    Sharipov, Sh.; Ermamatov, M. J. Bayimbetova, J. K.

    2008-02-15

    The properties of excited states of two deformable odd nuclei are investigated within the nonadiabatic model previously developed by the present authors. The results of relevant calculations are compared with available experimental data.

  8. Response of hot nuclei

    SciTech Connect

    Broglia, R.A.

    1986-01-01

    The dipole giant resonance is reviewed, as it is the only vibration which has been experimentally identified in the decay of hot nuclei. The mechanism of exciting the resonance and the mode of the resonance are described. The methods used to calculate the vibrations from the shell model are discussed, including the Hartree-Fock approximation and random phase approximation. Nuclei formed by compound nuclear reactions, which possess high excitation energy and angular momentum, are considered. It is argued that the stability of the dipole may be used to advantage in the study of other properties of nuclei at high excitation. It is also considered possible that the discussion of the dipole giant resonance may be extended to the gamma decay of the isovector quadrupole vibration. 26 refs., 18 figs. (LEW)

  9. Systematics of the first 2{sup +} excitation in spherical nuclei with the Skyrme quasiparticle random-phase approximation

    SciTech Connect

    Terasaki, J.; Engel, J.; Bertsch, G. F.

    2008-10-15

    We use the quasiparticle random-phase approximation (QRPA) and the Skyrme interactions SLy4 and SkM* to systematically calculate energies and transition strengths for the lowest 2{sup +} state in spherical even-even nuclei. The SkM* functional, applied to 178 spherical nuclei between Z=10 and 90, produces excitation energies that are on average 11% higher than experimental values, with residuals that fluctuate about the average by -35% to +55%. The predictions of SkM* and SLy4 have significant differences, in part because of differences in the calculated ground state deformations; SkM* performs better in both the average and dispersion of energies. Comparing the QRPA results with those of generator-coordinate-method (GCM) calculations, we find that the QRPA reproduces trends near closed shells better than the GCM, and that it overpredicts the energies less severely in general.

  10. Superdeformed nuclei: Shells-vs-liquid drop, pairing-vs-thermal excitations, triaxial-vs-octupole shapes, super-superdeformation

    SciTech Connect

    Dudek, J.

    1987-01-01

    Mechanisms influencing the behavior of superdeformed nuclei are studied using several well established nuclear structure techniques. In particular: pairing, thermal excitation, shell and liquid-drop mechanisms are considered. The effects of quadrupole and hexadecapole (both axial and non-axial), and octupole deformation degrees of freedom are studied. Most of the results are illustrated using the case of /sup 152/Dy nucleus in which a superdeformed band extending up to I approx. 60 h-bar has been found in experiment. Some comparisons between /sup 152/Dy and the nuclei in the neighborhood are given. Calculations show that pairing ''de-aligns'' typically 6 to 8 units of angular momentum, as compared to the corresponding rigid rotation. This takes place for spins extending up to the highest limit, and thus diminishes the effective moments of inertia. Predicted octupole shape susceptibility is extremely large, significantly stronger than the susceptibilities known in the ground-states of many Actinide nuclei. Consequences of this result for the near-constancy of the dynamical moments of inertia are pointed out. Nuclear level densities calculated in function of spin, excitation energy and deformation explain the ''unusual'' side feeding pattern of the /sup 152/Dy superdeformed states. Predictions of super-superdeformed nuclear states (axis ratio varying between 2:1 and 3:1 or more) are given and exemplified for Erbium nuclei. Finally, the problem of superdeformation stability and the influence of increased collective inertia on a barrier penetration are examined. An analytical expression for the effective inertia parameter is obtained and its derivation outlined. 35 refs., 9 figs.

  11. Identification of excited structures in proton unbound nuclei 173,175,177Au: shape co-existence and intruder bands

    NASA Astrophysics Data System (ADS)

    Kondev, F. G.; Carpenter, M. P.; Janssens, R. V. F.; Abu Saleem, K.; Ahmad, I.; Amro, H.; Cizewski, J. A.; Danchev, M.; Davids, C. N.; Hartley, D. J.; Heinz, A.; Khoo, T. L.; Lauritsen, T.; Lister, C. J.; Ma, W. C.; Poli, G. L.; Ressler, J.; Reviol, W.; Riedinger, L. L.; Seweryniak, D.; Smith, M. B.; Wiedenhöver, I.

    2001-07-01

    Excited states in the proton-unbound 173,175,177Au nuclei were identified for the first time. Level structures associated with three different shapes were observed in 175Au. While the yrast lines of 175Au and 177Au consist of a prolate band built upon the intruder 1/2+[660] (i13/2) proton orbital, no sign of collectivity was observed in the lighter 173Au isotope. Implications for the deformation associated with these structures are discussed with a focus on shape co-existence in the vicinity of the proton-drip line.

  12. The reduced transition probabilities for excited states of rare-earths and actinide even-even nuclei

    SciTech Connect

    Ghumman, S. S.

    2015-08-28

    The theoretical B(E2) ratios have been calculated on DF, DR and Krutov models. A simple method based on the work of Arima and Iachello is used to calculate the reduced transition probabilities within SU(3) limit of IBA-I framework. The reduced E2 transition probabilities from second excited states of rare-earths and actinide even–even nuclei calculated from experimental energies and intensities from recent data, have been found to compare better with those calculated on the Krutov model and the SU(3) limit of IBA than the DR and DF models.

  13. Comparison of DD, DT and Cf-252 neutron excitation of light and medium mass nuclei for field PGNAA applications

    NASA Astrophysics Data System (ADS)

    Seabury, E. H.; Blackburn, B. W.; Chichester, D. L.; Wharton, C. J.; Caffrey, A. J.

    2007-08-01

    Prompt Gamma Ray Neutron activation analysis can offer significant cost and safety advantages in the identification of explosives and toxic chemicals. As an example, the US military examined over a thousand suspect chemical munitions with Idaho National Laboratory's PINS Chemical Assay System last year. PGNAA requires, of course, a neutron source to excite the atomic nuclei of the item under test via neutron capture and inelastic neutron scattering reactions and the choice of neutron source can drastically affect PGNAA system performance. We have carried out Monte Carlo and laboratory experiments comparing DD, DT and Cf-252 neutrons incident on light and medium mass chemical elements, toward optimizing the design of future neutron-generator-based PGNAA systems for field use. We report the excitation of (n, γ) and (n, n‧) gamma rays from these elements by each type of neutron source.

  14. Evolution of collectivity near mid-shell from excited-state lifetime measurements in rare earth nuclei

    NASA Astrophysics Data System (ADS)

    Werner, V.; Cooper, N.; Régis, J.-M.; Rudigier, M.; Williams, E.; Jolie, J.; Cakirli, R. B.; Casten, R. F.; Ahn, T.; Anagnostatou, V.; Berant, Z.; Bonett-Matiz, M.; Elvers, M.; Heinz, A.; Ilie, G.; Radeck, D.; Savran, D.; Smith, M. K.

    2016-03-01

    The B (E 2 ) excitation strength of the first excited 2+ state in even-even nuclei should directly correlate with the size of the valence space and maximize at mid-shell. A previously found saturation of B (E 2 ) strengths in well-deformed rotors at mid-shell is tested through high-precision measurements of the lifetimes of the lowest-lying 2+ states of the 168Hf and 174W rare earth isotopes. Measurements were performed using fast LaBr3 scintillation detectors. Combined with the recently remeasured B (E 2 ;21+→01+) values for Hf and W isotopes the new data remove discrepancies observed in the differentials of B (E 2 ) values for these isotopes.

  15. NpNn dependence of empirical formula for the lowest excitation energy of the 2+ states in even even nuclei

    NASA Astrophysics Data System (ADS)

    Jin, Guanghao; Yoon, Jin-Hee; Cha, Dongwoo

    2008-03-01

    We examine the effects of the additional term of the type {\\sim} e^{- \\lambda^{\\prime} N_pN_n} on the recently proposed empirical formula for the lowest excitation energy of the 2+ states in even-even nuclei. This study is motivated by the fact that this term carries the favorable dependence of the valence nucleon numbers dictated by the NpNn scheme. We show explicitly that there is not any improvement in reproducing Ex(2+1) by including the extra NpNn term. However, our study also reveals that the excitation energies Ex(2+1), when calculated by the NpNn term alone (with the mass number A dependent term), are quite comparable to those calculated by the original empirical formula.

  16. Prediction of cloud condensation nuclei activity for organic compounds using functional group contribution methods

    DOE PAGESBeta

    Petters, M. D.; Kreidenweis, S. M.; Ziemann, P. J.

    2016-01-19

    A wealth of recent laboratory and field experiments demonstrate that organic aerosol composition evolves with time in the atmosphere, leading to changes in the influence of the organic fraction to cloud condensation nuclei (CCN) spectra. There is a need for tools that can realistically represent the evolution of CCN activity to better predict indirect effects of organic aerosol on clouds and climate. This work describes a model to predict the CCN activity of organic compounds from functional group composition. Following previous methods in the literature, we test the ability of semi-empirical group contribution methods in Köhler theory to predict themore » effective hygroscopicity parameter, kappa. However, in our approach we also account for liquid–liquid phase boundaries to simulate phase-limited activation behavior. Model evaluation against a selected database of published laboratory measurements demonstrates that kappa can be predicted within a factor of 2. Simulation of homologous series is used to identify the relative effectiveness of different functional groups in increasing the CCN activity of weakly functionalized organic compounds. Hydroxyl, carboxyl, aldehyde, hydroperoxide, carbonyl, and ether moieties promote CCN activity while methylene and nitrate moieties inhibit CCN activity. The model can be incorporated into scale-bridging test beds such as the Generator of Explicit Chemistry and Kinetics of Organics in the Atmosphere (GECKO-A) to evaluate the evolution of kappa for a complex mix of organic compounds and to develop suitable parameterizations of CCN evolution for larger-scale models.« less

  17. Prediction of cloud condensation nuclei activity for organic compounds using functional group contribution methods

    DOE PAGESBeta

    Petters, M. D.; Kreidenweis, S. M.; Ziemann, P. J.

    2016-01-19

    A wealth of recent laboratory and field experiments demonstrate that organic aerosol composition evolves with time in the atmosphere, leading to changes in the influence of the organic fraction to cloud condensation nuclei (CCN) spectra. There is a need for tools that can realistically represent the evolution of CCN activity to better predict indirect effects of organic aerosol on clouds and climate. This work describes a model to predict the CCN activity of organic compounds from functional group composition. Following previous methods in the literature, we test the ability of semi-empirical group contribution methods in Kohler theory to predict themore » effective hygroscopicity parameter, kappa. However, in our approach we also account for liquid–liquid phase boundaries to simulate phase-limited activation behavior. Model evaluation against a selected database of published laboratory measurements demonstrates that kappa can be predicted within a factor of 2. Simulation of homologous series is used to identify the relative effectiveness of different functional groups in increasing the CCN activity of weakly functionalized organic compounds. Hydroxyl, carboxyl, aldehyde, hydroperoxide, carbonyl, and ether moieties promote CCN activity while methylene and nitrate moieties inhibit CCN activity. Furthermore, the model can be incorporated into scale-bridging test beds such as the Generator of Explicit Chemistry and Kinetics of Organics in the Atmosphere (GECKO-A) to evaluate the evolution of kappa for a complex mix of organic compounds and to develop suitable parameterizations of CCN evolution for larger-scale models.« less

  18. Prediction of cloud condensation nuclei activity for organic compounds using functional group contribution methods

    NASA Astrophysics Data System (ADS)

    Petters, M. D.; Kreidenweis, S. M.; Ziemann, P. J.

    2016-01-01

    A wealth of recent laboratory and field experiments demonstrate that organic aerosol composition evolves with time in the atmosphere, leading to changes in the influence of the organic fraction to cloud condensation nuclei (CCN) spectra. There is a need for tools that can realistically represent the evolution of CCN activity to better predict indirect effects of organic aerosol on clouds and climate. This work describes a model to predict the CCN activity of organic compounds from functional group composition. Following previous methods in the literature, we test the ability of semi-empirical group contribution methods in Köhler theory to predict the effective hygroscopicity parameter, kappa. However, in our approach we also account for liquid-liquid phase boundaries to simulate phase-limited activation behavior. Model evaluation against a selected database of published laboratory measurements demonstrates that kappa can be predicted within a factor of 2. Simulation of homologous series is used to identify the relative effectiveness of different functional groups in increasing the CCN activity of weakly functionalized organic compounds. Hydroxyl, carboxyl, aldehyde, hydroperoxide, carbonyl, and ether moieties promote CCN activity while methylene and nitrate moieties inhibit CCN activity. The model can be incorporated into scale-bridging test beds such as the Generator of Explicit Chemistry and Kinetics of Organics in the Atmosphere (GECKO-A) to evaluate the evolution of kappa for a complex mix of organic compounds and to develop suitable parameterizations of CCN evolution for larger-scale models.

  19. Prediction of cloud condensation nuclei activity for organic compounds using functional group contribution methods

    SciTech Connect

    Petters, M. D.; Kreidenweis, S. M.; Ziemann, P. J.

    2016-01-01

    A wealth of recent laboratory and field experiments demonstrate that organic aerosol composition evolves with time in the atmosphere, leading to changes in the influence of the organic fraction to cloud condensation nuclei (CCN) spectra. There is a need for tools that can realistically represent the evolution of CCN activity to better predict indirect effects of organic aerosol on clouds and climate. This work describes a model to predict the CCN activity of organic compounds from functional group composition. Following previous methods in the literature, we test the ability of semi-empirical group contribution methods in Köhler theory to predict the effective hygroscopicity parameter, kappa. However, in our approach we also account for liquid–liquid phase boundaries to simulate phase-limited activation behavior. Model evaluation against a selected database of published laboratory measurements demonstrates that kappa can be predicted within a factor of 2. Simulation of homologous series is used to identify the relative effectiveness of different functional groups in increasing the CCN activity of weakly functionalized organic compounds. Hydroxyl, carboxyl, aldehyde, hydroperoxide, carbonyl, and ether moieties promote CCN activity while methylene and nitrate moieties inhibit CCN activity. The model can be incorporated into scale-bridging test beds such as the Generator of Explicit Chemistry and Kinetics of Organics in the Atmosphere (GECKO-A) to evaluate the evolution of kappa for a complex mix of organic compounds and to develop suitable parameterizations of CCN evolution for larger-scale models.

  20. Prediction of cloud condensation nuclei activity for organic compounds using functional group contribution methods

    NASA Astrophysics Data System (ADS)

    Petters, M. D.; Kreidenweis, S. M.; Ziemann, P. J.

    2015-09-01

    A wealth of recent laboratory and field experiments demonstrate that organic aerosol composition evolves with time in the atmosphere, leading to changes in the influence of the organic fraction to cloud condensation nuclei (CCN) spectra. There is a need for tools that can realistically represent the evolution of CCN activity to better predict indirect effects of organic aerosol on clouds and climate. This work describes a model to predict the CCN activity of organic compounds from functional group composition. The model combines Köhler theory with semi-empirical group contribution methods to estimate molar volumes, activity coefficients and liquid-liquid phase boundaries to predict the effective hygroscopicity parameter, kappa. Model evaluation against a selected database of published laboratory measurements demonstrates that kappa can be predicted within a factor of two. Simulation of homologous series is used to identify the relative effectiveness of different functional groups in increasing the CCN activity of weakly functionalized organic compounds. Hydroxyl, carboxyl, aldehyde, hydroperoxide, carbonyl, and ether moieties promote CCN activity while methylene and nitrate moieties inhibit CCN activity. The model can be incorporated into scale-bridging testbeds such as the Generator of Explicit Chemistry and Kinetics of Organics in the Atmosphere to evaluate the evolution of kappa for a complex mix of organic compounds and to develop suitable parameterizations of CCN evolution for larger scale models.

  1. Emission of complex fragments for compound nuclei formed far from the stability line for A{approx}120

    SciTech Connect

    Gomez Del Campo, J.

    1996-10-01

    Experiments and calculations are presented for the emission of complex fragments (Z>2) from compound nuclei around mass 120 and for bombarding energies below 15 MeV/nucleon. It is shown that a strong enhancement in the emission of complex fragments (especially for Z=6) is expected for compound nuclei formed close or at the N=Z line. Several predictions are given that could be tested with the radioactive beams soon to be available. Also results from a recent experiment that utilizes the emission of complex fragments for {gamma}-ray nuclear spectroscopy studies are presented.

  2. ALERT I and II: Hauser Feshbach codes for nuclei at high excitation and angular momenta

    SciTech Connect

    Blann, M; Komoto, T A

    1982-05-01

    A description is given of two versions of a Hauser Feshbach code descended from the MBII code. The level density options, which include collective enhancement options, modeling of transmission coefficients for deformed nuclei, and fission barrier options are discussed in some detail. A listing of the codes, plus sample input and output are appended.

  3. Dynamical Model for the Decay of Hot and Rotating Compound Nuclei

    SciTech Connect

    Gupta, Raj K.; Singh, Dalip; Arun, Sham K.; Niyti; Kumar, Raj

    2009-03-04

    As an alternative to the well known Hauser-Feshbach analysis and statistical fission model, a dynamical collective clusterization model, called the dynamical cluster-decay model (DCM), is developed for the decay of hot and rotating compound nuclei (CN) formed in the low-energy heavy ion reactions. The model is a non-statistical description for the decay of a CN to light particles (LPs), intermediate mass fragments (IMFs), fusion-fission (FF) and quasi-fission (QF)(equivalently, capture) processes. The model considers all decay products as dynamical mass motions of preformed fragments or clusters through the interaction barrier, thereby including structure effects of the CN, and is applicable to CN from different mass regions.

  4. Electric quadrupole excitations in the interactions of Y-89 with relativistic nuclei

    NASA Technical Reports Server (NTRS)

    Norbury, John W.

    1989-01-01

    The first complete calculations of electric quadrupole excitations in relativistic nucleus-nucleus collisions are presented herein. Neutron emission from Y-89 is studied and quadrupole effects are found to be a significant fraction of the cross section.

  5. Single-phonon and multi-phonon excitations of the γ vibration in rotating odd-A nuclei

    NASA Astrophysics Data System (ADS)

    Matsuzaki, Masayuki

    2014-10-01

    Background: Collective motions in quantum many-body systems are described as bosonic excitations. Multi-phonon excitations in atomic nuclei, however, were observed very rarely. In particular, the first two-phonon γ vibrational (2γ) excitation in odd-A nuclei was reported in 2006 and only a few have been known so far. Two theoretical calculations for the data on Nb103 were performed, one of which was done by the present author within a limited model space up to 2γ basis states. Quite recently, conspicuously enhanced B (E2)s, reduced E2 transition probabilities, feeding 2γ states were observed in Nb105 and conjectured that their parent states, called band (4), are candidates of 3γ states. Purpose: In the present work, the model space is enlarged up to 4γ basis states. The purpose is twofold: One is to see how the description of 2γ eigenstates in the previous work is improved, and the other is to examine the existence of collective 3γ eigenstates, and when they exist, study their collectivity through calculating interband B (E2)s. Method: The particle-vibration coupling model based on the cranking model and the random-phase approximation is used to calculate the vibrational states in rotating odd-A nuclei. Interband B (E2)s are calculated by adopting the method of the generalized intensity relation. Results: The present model reproduces well the energy spectra and B (E2)s of 0γ-2γ states in Nb103 and Nb105. For 3γ states, calculated spectra indicate that the most collective state with the highest K at zero rotation feels strong Coriolis force after rotation sets in and consequently is observed with lowered K, where K is the projection of the angular momentum to the z axis. The calculated states account for the observed enhanced B (E2)s within factors of 2-3. Conclusions: The present calculation with the enlarged model space reproduces the observed 0γ-2γ states well and predicts properties of collective 3γ states. The most collective one is thought to be

  6. Statistical Properties of Excited Nuclei in the Mass Range 47≤A≤59

    NASA Astrophysics Data System (ADS)

    Zhuravlev, B. V.; Lychagin, A. A.; Titarenko, N. N.; Demenkov, V. G.; Trykova, V. I.

    2012-02-01

    Level densities and their energy dependences for nuclei in the mass range 47≤A≤59 have been determined from the measurements of neutron evaporation spectra in (p,n) reaction. Neutron spectra from (p,n) reaction on nuclei of 47Ti, 48Ti, 49Ti, 53Cr, 54Cr, 57Fe, 59Co have been measured at proton energies between 7 and 11 MeV. The measurements of neutron spectra were performed by time-of-flight fast neutron spectrometer on the pulsed tandem accelerator EGP-15 of IPPE. The high resolution and stability of time-of-flight spectrometer allowed identify reliably the discrete low-lying levels together with continuum part of neutron spectra. Analyses of the measured data have been carried out in the framework of statistical equilibrium and pre-equilibrium models of nuclear reactions. The calculations are done with use of the exact formalism of the statistical theory as given by Hauser-Feshbach with the generalized superfluid model of nucleus, the back-shifted Fermi-gas model and the composite formula of Gilbert-Cameron for nuclear level density. The nuclear level densities of 47V, 48V, 49V, 53Mn, 54Mn, 57Co, 59Ni and their energy dependences have been determined. The obtained results have been discussed in totality with existing experimental and model systematic data.

  7. Statistical properties of excited nuclei in the mass range 47 ⩽ A ⩽ 59

    NASA Astrophysics Data System (ADS)

    Zhuravlev, B. V.; Lychagin, A. A.; Titarenko, N. N.; Demenkov, V. G.; Trykova, V. I.

    2012-09-01

    Level densities and their energy dependences for nuclei in the mass range of 47 ≤ A ≤ 59 were determined from the results obtained by measuring neutron-evaporation spectra in respective ( p, n) reactions. The spectra of neutrons originating from the ( p, n) reactions on 47Ti, 48Ti, 49Ti, 53Cr, 54Cr, 57Fe, and 59Co nuclei were measured in the proton-energy range of 7-11 MeV. These measurements were performed with the aid of a fast-neutron spectrometer by the time-of-flight method over the base of the EGP-15 pulsed tandem accelerator installed at the Institute for Physics and Power Engineering (Obninsk, Russia). A high resolution of the spectrometer and its stability in the time of flight made it possible to identify reliably discrete low-lying levels along with the continuum part of neutron spectra. Our measured data were analyzed within the statistical equilibrium and preequilibrium models of nuclear reactions. The respective calculations were performed with the aid of the Hauser-Feshbach formalismof statistical theory supplemented with the generalized model of a superfluid nucleus, the back-shifted Fermi gas model, and the Gilbert-Cameron composite formula for nuclear level densities. Nuclear level densities for 47V, 48V, 49V, 53Mn, 54Mn, 57Co, and 59Ni and their energy dependences were determined. The results are discussed and compared with available experimental data and with recommendations of model-based systematics.

  8. Using LaBr3(Ce) Detectors for Precision Lifetime Measurements of Excited States in `Interesting' Nuclei

    NASA Astrophysics Data System (ADS)

    Regan, P. H.

    2015-11-01

    Precision measurements of electromagnetic transition rates provide accurate inputs into nuclear data evaluations and are also used to test and validate predictions of state of the art nuclear structure models. Measurements of transition rates can be used to ascertain or rule out multipolarity assignments for the measured EM decay, thereby providing spin- and parity-difference information for states between which the EM transition takes place. This conference paper reports on a measurements of electromagnetic transition rates between excited nuclear states using coincidence `fast-timing' gamma-ray spectroscopy with cerium-doped, lanthanum-tribromide (LaBr3(Ce)) detectors. Examples of recent precision measurements using a combined LaBr3-HpGe array based at the tandem accelerator, Bucharest, Romania include studies around the N=20 and N=82 shell closures using stable-beam induced fusion-evaporation reactions; and the evolution of nuclear deformation around in neutron-rich Hf, W and Os nuclei using 7Li-induced light-ion transfer reactions. This paper also presents the ongoing development of a new multidetector LaBr3(Ce) array for future studies of exotic nuclei produced at the upcoming Facility for Anti-Proton and Ion Research (FAIR) as part of the NUSTAR-DESPEC project, and reports on the pre-NUSTAR implementations of detectors from this array to study electromagnetic transition rates in neutron-rich fission fragments at ILL-Grenoble, France and RIBF at RIKEN, Japan.

  9. Charge-changing particle-hole excitation of 16N and 16F nuclei

    NASA Astrophysics Data System (ADS)

    Taqi Al-Bayati, Ali H.; Darwesh, Sarah S.

    2013-12-01

    The nuclear structure of 16N (closed shell + ν - π) and 16F (closed shell + π - ν) nuclei is studied using particle-hole proton-neutron Tamm-Dancoff Approximation pn TDA and particle-hole proton-neutron Random Phase Approximation pn RPA. The particle-hole Hamiltonian of PSD model space is to be diagonalized in the presence of the PSDMWKPN interaction: for P-space the Cohen-Kurath interaction, for SD-space the Wildenthal Interaction, for the coupling matrix elements between P- and SD-spaces the Millener-Kurath interaction is used, spurious components were eliminated with CM contribution. The results containing energy level schemes and electromagnetic transition strength are compared with the available experimental data.

  10. Charge-changing particle-hole excitation of {sup 16}N and {sup 16}F nuclei

    SciTech Connect

    Taqi Al-Bayati, Ali H.; Darwesh, Sarah S.

    2013-12-16

    The nuclear structure of {sup 16}N (closed shell + ν − π) and {sup 16}F (closed shell + π − ν) nuclei is studied using particle-hole proton-neutron Tamm-Dancoff Approximation pn TDA and particle-hole proton-neutron Random Phase Approximation pn RPA. The particle-hole Hamiltonian of PSD model space is to be diagonalized in the presence of the PSDMWKPN interaction: for P-space the Cohen-Kurath interaction, for SD-space the Wildenthal Interaction, for the coupling matrix elements between P- and SD-spaces the Millener-Kurath interaction is used, spurious components were eliminated with CM contribution. The results containing energy level schemes and electromagnetic transition strength are compared with the available experimental data.

  11. Exciting fluorescence compounds on an optical fiber's side surface with a liquid core waveguide.

    PubMed

    Ray, Jason C; Almas, Muhammad S; Tao, Shiquan

    2016-01-01

    A new fiber optic fluorescence spectroscopic method using a liquid core waveguide (LCW) as an excitation element has been developed for detecting a fluorescence compound absorbed on an optical fiber's surface. A laser light beam was coupled into a multimode optical fiber. The distal end of the fiber was inserted into an LCW. The diverging light emerging from the fiber's end was collected and guided within the LCW. A tapered optical fiber was inserted into the LCW from the other side. Laser light traveling in the LCW evenly illuminates the tapered fiber surface and excites fluorescence molecules absorbed on the tapered fiber's surface. Fluorescence light emitted from the tapered fiber surface was collected with the fiber itself and delivered through the fiber to an optical fiber compatible spectrometer for detection. This new technique provides an efficient way for evenly exciting fluorescence compounds absorbed on an optical fiber's surface. PMID:26696168

  12. Study of two-photon excitation spectra of organic compounds absorbing in the UV region

    SciTech Connect

    Babenko, V A; Sychev, Andrei A

    2004-12-31

    A method is proposed for recording two-photon excitation (TPE) spectra of organic compounds with the help of picosecond pulses from a dye laser tunable in the range from 550 to 640 nm. The TPE spectra are obtained for organic scintillators and drugs: paraterphenyl in liquid and solid phases, stilbene single crystal and Streptocid powder, having a one-photon absorption band in the region from 270 to 350 nm. It is shown that the vibronic structure in the TPE spectra of these compounds is independent of their aggregate state and is an individual characteristic of each of the compounds. (active media)

  13. Nonquenched Isoscalar Spin-M1 Excitations in sd-Shell Nuclei.

    PubMed

    Matsubara, H; Tamii, A; Nakada, H; Adachi, T; Carter, J; Dozono, M; Fujita, H; Fujita, K; Fujita, Y; Hatanaka, K; Horiuchi, W; Itoh, M; Kawabata, T; Kuroita, S; Maeda, Y; Navrátil, P; von Neumann-Cosel, P; Neveling, R; Okamura, H; Popescu, L; Poltoratska, I; Richter, A; Rubio, B; Sakaguchi, H; Sakaguchi, S; Sakemi, Y; Sasamoto, Y; Shimbara, Y; Shimizu, Y; Smit, F D; Suda, K; Tameshige, Y; Tokieda, H; Yamada, Y; Yosoi, M; Zenihiro, J

    2015-09-01

    Differential cross sections of isoscalar and isovector spin-M1 (0(+)→1(+)) transitions are measured using high-energy-resolution proton inelastic scattering at E(p)=295  MeV on (24)Mg, (28)Si, (32)S, and (36)Ar at 0°-14°. The squared spin-M1 nuclear transition matrix elements are deduced from the measured differential cross sections by applying empirically determined unit cross sections based on the assumption of isospin symmetry. The ratios of the squared nuclear matrix elements accumulated up to E(x)=16  MeV compared to a shell-model prediction are 1.01(9) for isoscalar and 0.61(6) for isovector spin-M1 transitions, respectively. Thus, no quenching is observed for isoscalar spin-M1 transitions, while the matrix elements for isovector spin-M1 transitions are quenched by an amount comparable with the analogous Gamow-Teller transitions on those target nuclei. PMID:26382672

  14. Deformation increase of high-spin core-excited isomers in the astatine nuclei

    SciTech Connect

    Scheveneels, G.; Hardeman, F.; Neyens, G.; Coussement, R. )

    1991-06-01

    Quadrupole moments of six high-spin isomers in the At isotopes have been measured with the level-mixing-spectroscopy method: {sup 208}At(16{sup {minus}}), {sup 209}At(29/2{sup +}), {sup 210}At(19{sup +},15{sup {minus}}), {sup 211}At(39/2{sup {minus}},29/2{sup +}). The results show that level mixing spectroscopy is a promising technique to determine quadrupole moments of isomers that are difficult to measure by other in-beam hyperfine interaction methods. A large increase of the quadrupole moment is observed if neutrons are excited across or removed from the {ital N}=126 shell closure. This behavior is explained in terms of an enhanced core softness for fewer core neutrons; the aligned valence particles, moving in equatorial orbits, then easily polarize the core towards oblate deformation.

  15. Charge-exchange modes of excitation in deformed neutron-rich nuclei

    SciTech Connect

    Yoshida, Kenichi

    2015-10-15

    Gamow-Teller (GT) mode of excitation and β-decay properties of deformed neutron-rich even-N Zr isotopes are investigated in a self-consistent Skyrme energy-density-functional approach, in which the Hartree-Fock-Bogoliubov equation is solved in the coordinate space and the proton-neutron Quasiparticle-RPA equation is solved in the quasiparticle basis. It is found that a stronger collectivity is generated for the GT giant resonance as an increase in the neutron number. Furthermore, we find that the T = 0 pairing enhances the low-lying GT strengths cooperatively with the T = 1 pairing correlation depending on the microscopic structure of the low-lying mode and the shell structure around the Fermi levels, and that the enhanced strength shortens the β-decay half-lives by at most an order of magnitude.

  16. Possible conservation of the K-quantum number in excited rotating nuclei

    SciTech Connect

    Bracco, A.; Bosetti, P.; Leoni, S. |

    1996-12-31

    The {gamma}-cascades feeding into low-K and high-K bands in the nucleus {sup 163}Er are investigated by analyzing variances and covariances of the spectrum fluctuations. The study of the covariance between pairs of gated spectra reveals that the cascades feeding into the low-K bands are completely different from those feeding the high-K bands. In addition, the number of decay paths obtained analyzing the ridge and the valley in spectra gated by high-K transitions is different than that deduced from the total spectrum. This result is well reproduced with microscopic calculations of strongly interacting bands. It is concluded that the K-selection rules are effective for the excited rotational bands within the angular momentum region probed by the experiment, 30{Dirac_h} {le} I {le} 40{Dirac_h}.

  17. Role of nuclear couplings in the inelastic excitation of weakly-bound neutron-rich nuclei

    SciTech Connect

    Dasso, C.H.; Lenzi, S.M.; Vitturi, A.

    1996-12-31

    Much effort is presently devoted to the study of nuclear systems far from the stability line. Particular emphasis has been placed in light systems such as {sup 11}Li, {sup 8}B and others, where the very small binding energy of the last particles causes their density distribution to extend considerably outside of the remaining nuclear core. Some of the properties associated with this feature are expected to characterize also heavier systems in the vicinity of the proton or neutron drip lines. It is by now well established that low-lying concentrations of multipole strength arise from pure configurations in which a peculiar matching between the wavelength of the continuum wavefunction of the particles and the range of the weakly-bound hole states occurs. To this end the authors consider the break-up of a weakly-bound system in a heavy-ion collision and focus attention in the inelastic excitation of the low-lying part of the continuum. They make use of the fact that previous investigations have shown that the multipole response in this region is not of a collective nature and describe their excited states as pure particle-hole configurations. Since the relevant parameter determining the strength distributions is the binding energy of the last bound orbital they find it most convenient to use single-particle wavefunctions generated by a sperical square-well potential with characteristic nuclear dimensions and whose depth has been adjusted to give rise to a situation in which the last occupied neutron orbital is loosely-bound. Spin-orbit couplings are, for the present purpose, ignored. The results of this investigation clearly indicate that nuclear couplings have the predominant role in causing projectile dissociation in many circumstances, even at bombarding energies remarkably below the Coulomb barrier.

  18. How To Reach Intense Luminescence for Compounds Capable of Excited-State Intramolecular Proton Transfer?

    PubMed

    Skonieczny, Kamil; Yoo, Jaeduk; Larsen, Jillian M; Espinoza, Eli M; Barbasiewicz, Michał; Vullev, Valentine I; Lee, Chang-Hee; Gryko, Daniel T

    2016-05-23

    Photoinduced intramolecular direct arylation allows structurally unique compounds containing phenanthro[9',10':4,5]imidazo[1,2-f]phenanthridine and imidazo[1,2-f]phenanthridine skeletons, which mediate excited-state intramolecular proton transfer (ESIPT), to be efficiently synthesized. The developed polycyclic aromatics demonstrate that the combination of five-membered ring structures with a rigid arrangement between a proton donor and a proton acceptor provides a means for attaining large fluorescence quantum yields, exceeding 0.5, even in protic solvents. Steady-state and time-resolved UV/Vis spectroscopy reveals that, upon photoexcitation, the prepared protic heteroaromatics undergo ESIPT, converting them efficiently into their excited-state keto tautomers, which have lifetimes ranging from about 5 to 10 ns. The rigidity of their structures, which suppresses nonradiative decay pathways, is believed to be the underlying reason for the nanosecond lifetimes of these singlet excited states and the observed high fluorescence quantum yields. Hydrogen bonding with protic solvents does not interfere with the excited-state dynamics and, as a result, there is no difference between the occurrences of ESIPT processes in MeOH versus cyclohexane. Acidic media has a more dramatic effect on suppressing ESIPT by protonating the proton acceptor. As a result, in the presence of an acid, a larger proportion of the fluorescence of ESIPT-capable compounds originates from their enol excited states. PMID:27062363

  19. Singlet-Triplet Excitations in the Unconventional Spin-Peierls TiOBr Compound

    NASA Astrophysics Data System (ADS)

    Clancy, J. P.; Gaulin, B. D.; Adams, C. P.; Granroth, G. E.; Kolesnikov, A. I.; Sherline, T. E.; Chou, F. C.

    2011-03-01

    We have performed time-of-flight neutron scattering measurements on powder samples of the unconventional spin-Peierls compound TiOBr using the fine-resolution Fermi chopper spectrometer (SEQUOIA) at the Spallation Neutron Source at Oak Ridge National Laboratory. These measurements reveal two branches of magnetic excitations within the commensurate and incommensurate spin-Peierls phases, which we associate with n=1 and n=2 triplet excitations out of the singlet ground state. These results represent the first direct measurement of the singlet-triplet energy gap in TiOBr, which has a value of Eg=21.2±1.0meV.

  20. Characterization of the multifragment decay channel in highly excited nuclei. [Indiana Univ. , Bloomington, Indiana

    SciTech Connect

    de Souza, R.T.

    1992-10-01

    Characteristics of multifragment decay in heavy-ion induced reactions at intermediate energies are explored. Evolution of the timescale for emission of intermediate mass fragments (IMF: 3[le]Z[le]20) is investigated. Fragments associated with central collisions in the reactions [sup 36]Ar + [sup 197]Au at E/A = 50, 80, and 110 MeV are emitted on an extremely fast timescale, [tau] [le] 75 fm/c, comparable to the transit time of the projectile past the target nucleus. With increasing incident energy, mean fragment emission times decrease, consistent with statistical decay from highly excited systems or fast dynamical processes. To examine the importance of expansion effects in multifragmentation, the transverse kinetic energy of fragments was investigated. Evidence for expansion effects in the system [sup 36]Ar + [sup 197]Au at E/A = 50, 80, and 110 MeV was indicated by the charge dependence of the mean isotropic kinetic energy. At the highest incident energy the data suggest the onset of volume emission. Construction and performance of low-threshold high-resolution detector telescopes is discussed. Three-body Coulomb trajectory calculations are being used to probe kinematical correlations associated with neck emission of IMFs during fission. Initial design and testing of position sensitive parallel plate avalanche counters for upcoming ternary fission experiments is discussed.

  1. Monitor RNA synthesis in live cell nuclei by using two-photon excited fluorescence lifetime imaging microscopy

    NASA Astrophysics Data System (ADS)

    Peng, Xiao; Lin, Danying; Wang, Yan; Qi, Jing; Yan, Wei; Qu, Junle

    2015-03-01

    Probing of local molecular environment in cells is of significant value in creating a fundamental understanding of cellular processes and molecular profiles of diseases, as well as studying drug cell interactions. In order to investigate the dynamically changing in subcellular environment during RNA synthesis, we applied two-photon excited fluorescence lifetime imaging microscopy (FLIM) method to monitor the green fluorescent protein (GFP) fused nuclear protein ASF/SF2. The fluorescence lifetime of fluorophore is known to be in inverse correlation with a local refractive index, and thus fluorescence lifetimes of GFP fusions provide real-time information of the molecular environment of ASF/SF2- GFP. The FLIM results showed continuous and significant fluctuations of fluorescence lifetimes of the fluorescent protein fusions in live HeLa cells under physiological conditions. The fluctuations of fluorescence lifetime values indicated the variations of activities of RNA polymerases. Moreover, treatment with pharmacological drugs inhibiting RNA polymerase activities led to irreversible decreases of fluorescence lifetime values. In summary, our study of FLIM imaging of GFP fusion proteins has provided a sensitive and real-time method to investigate RNA synthesis in live cell nuclei.

  2. Band-head spectra of low-energy single-particle excitations in some well-deformed, odd-mass heavy nuclei within a microscopic approach

    NASA Astrophysics Data System (ADS)

    Koh, Meng-Hock; Duy Duc, Dao; Nhan Hao, T. V.; Thuy Long, Ha; Quentin, P.; Bonneau, L.

    2016-01-01

    In four well-deformed heavy odd nuclei, the energies of low-lying rotational band heads have been determined microscopically within a self-consistent Hartree-Fock-plus-BCS approach with blocking. A Skyrme nucleon-nucleon effective interaction has been used together with a seniority force to describe pairing correlations. Only such states which are phenomenologically deemed to be related to single-particle excitations have been considered. The polarization effects, including those associated with the genuine time-reversal symmetry breaking have been fully taken into account within our model assumptions. The calculated spectra are in reasonably good qualitative agreement with available data for the considered odd-neutron nuclei. This is not so much the case for the odd-proton nuclei. A potential explanation for such a difference in behavior is proposed.

  3. Nucleus Z=126 with magic neutron number N=184 may be related to the measured Maruhn-Greiner maximum at A/2=155 from compound nuclei at low energy nuclear reactions

    NASA Astrophysics Data System (ADS)

    Prelas, M. A.; Hora, H.; Miley, G. H.

    2014-07-01

    Evaluation of nuclear binding energies from theory close to available measurements of a very high number of superheavy elements (SHE) based on α-decay energies Qα, arrived at a closing shell with a significant neutron number 184. Within the option of several discussed magic numbers for protons of around 120, Bagge's numbers 126 and 184 fit well and are supported by the element generation measurements by low energy nuclear reactions (LENR) discovered in deuterium loaded host metals. These measurements were showing a Maruhn-Greiner maximum from fission of compound nuclei in an excited state with double magic numbers for mutual confirmation.

  4. Use of image analysis to estimate anthocyanin and UV-excited fluorescent phenolic compound levels in strawberry fruit

    PubMed Central

    Yoshioka, Yosuke; Nakayama, Masayoshi; Noguchi, Yuji; Horie, Hideki

    2013-01-01

    Strawberry is rich in anthocyanins, which are responsible for the red color, and contains several colorless phenolic compounds. Among the colorless phenolic compounds, some, such as hydroxycinammic acid derivatives, emit blue-green fluorescence when excited with ultraviolet (UV) light. Here, we investigated the effectiveness of image analyses for estimating the levels of anthocyanins and UV-excited fluorescent phenolic compounds in fruit. The fruit skin and cut surface of 12 cultivars were photographed under visible and UV light conditions; colors were evaluated based on the color components of images. The levels of anthocyanins and UV-excited fluorescent compounds in each fruit were also evaluated by spectrophotometric and high performance liquid chromatography (HPLC) analyses, respectively and relationships between these levels and the image data were investigated. Red depth of the fruits differed greatly among the cultivars and anthocyanin content was well estimated based on the color values of the cut surface images. Strong UV-excited fluorescence was observed on the cut surfaces of several cultivars, and the grayscale values of the UV-excited fluorescence images were markedly correlated with the levels of those fluorescent compounds as evaluated by HPLC analysis. These results indicate that image analyses can select promising genotypes rich in anthocyanins and fluorescent phenolic compounds. PMID:23853516

  5. Excitation energies and temperatures of hot nuclei produced in the reactions of {sup 63}Cu+{sup 197}Au at 35A MeV

    SciTech Connect

    Wada, R.; Tezkratt, R.; Hagel, K.; Haddad, F.; Kolomiets, A.; Lou, Y.; Li, J.; Shimooka, M.; Shlomo, S.; Utley, D.; Xiao, B.; Mdeiwayeh, N.; Natowitz, J.B.; Majka, Z.; Cibor, J.; Kozik, T.; Sosin, Z.

    1997-01-01

    Observations of heavy remnants emitted at forward angles with high velocities and high associated particle multiplicities have been used to select central collisions of 35A MeV {sup 63}Cu with {sup 197}Au. The data indicate that these remnants, both fission fragments and evaporation residuelike products, result from the deexcitation of nuclei with A{approximately}225{endash}240 having excitation energies of {approximately} 800{endash}1300 MeV. Similar particle multiplicities are observed for both evaporative and fission decay channels. Modeling the results with hybrid codes which treat entrance channel dynamics followed by sequential statistical decay requires the inclusion of some delay in the fission channel to produce heavy remnants with mass A{ge}130, but the trend of the predicted velocities of these heavy remnants is different from that of the experiments. Calculations with a dynamic model based on the molecular dynamics approach have also been performed and lead to similar results. He and Li isotope yield ratios and the apparent temperatures derived from those ratios are similar to those previously reported for excited nuclei in this mass region. Temperatures derived from other yield ratios are also similar once a self-consistent treatment, taking into account population and decay of known excited states, is applied. The derived temperatures show little variation with excitation energy, suggesting that a limiting temperature may be reached at relatively low excitation energy, although the interpretation of this result and the determination of the actual initial value of this temperature is model dependent. Comments on the application of the double isotope yield ratio technique to extraction of the nuclear caloric curve are made. {copyright} {ital 1997} {ital The American Physical Society}

  6. Compound-nuclear reactions with unstable nuclei: Constraining theory through innovative experimental approaches

    NASA Astrophysics Data System (ADS)

    Escher, J. E.; Tonchev, A. P.; Burke, J. T.; Bedrossian, P.; Casperson, R. J.; Cooper, N.; Hughes, R. O.; Humby, P.; Ilieva, R. S.; Ota, S.; Pietralla, N.; Scielzo, N. D.; Werner, V.

    2016-06-01

    Cross sections for compound-nuclear reactions involving unstable targets are important for many applications, but can often not be measured directly. Several indirect methods have recently been proposed to determine neutron capture cross sections for unstable isotopes. We consider three approaches that aim at constraining statistical calculations of capture cross sections with data obtained from the decay of the compound nucleus relevant to the desired reaction. Each method produces this compound nucleus in a different manner (via a light-ion reaction, a photon-induced reaction, or β-decay) and requires additional ingredients to yield the sought-after cross section. We give a brief outline of the approaches and employ preliminary results from recent measurements to illustrate the methods. We discuss the main advantages and challenges of each approach.

  7. Interweaving of elementary modes of excitation in superfluid nuclei through particle-vibration coupling: Quantitative account of the variety of nuclear structure observables

    NASA Astrophysics Data System (ADS)

    Idini, A.; Potel, G.; Barranco, F.; Vigezzi, E.; Broglia, R. A.

    2015-09-01

    A complete characterization of the structure of nuclei can be obtained by combining information arising from inelastic scattering, Coulomb excitation, and γ -decay, together with one- and two-particle transfer reactions. In this way it is possible to probe both the single-particle and collective components of the nuclear many-body wave function resulting from the coupling of these modes and, as a result, diagonalizing the low-energy Hamiltonian. We address the question of how accurately such a description can account for experimental observations in the case of superfluid nuclei. Our treatment goes beyond the traditional approach, in which these properties are calculated separately, and most often for systems near closed shells, based on perturbative approximations (weak coupling). It is concluded that renormalizing empirically and on equal footing bare single-particle and collective motion of open-shell nuclei in terms of self-energy (mass) and vertex corrections (screening), as well as particle-hole and pairing interactions through particle-vibration coupling (PVC), leads to a detailed, quantitative account of the data, constraining the possible values of the k mass, of the 1S0 bare N N interaction, and of the PVC strengths within a rather narrow window.

  8. Evidence for Cation-Controlled Excited-State Localization in a Ruthenium Polypyridyl Compound.

    PubMed

    Beauvilliers, Evan E; Meyer, Gerald J

    2016-08-01

    The visible absorption and photoluminescence (PL) properties of the four neutral ruthenium diimine compounds [Ru(bpy)2(dcb)] (B2B), [Ru(dtb)2(dcb)] (D2B), [Ru(bpy)2(dcbq)] (B2Q), and [Ru(dtb)2(dcbq)] (D2Q), where bpy is 2,2'-bipyridine, dcb is 4,4'-(CO2(-))2-bpy, dtb is 4,4'-(tert-butyl)2-bpy, and dcbq is 4,4'-(CO2(-))2-2,2'-biquinoline, are reported in the presence of Lewis acidic cations present in fluid solutions at room temperature. In methanol solutions, the measured spectra were insensitive to the presence of these cations, while in acetonitrile a significant red shift in the PL spectra (≤1400 cm(-1)) was observed consistent with stabilization of the metal-to-ligand charge transfer (MLCT) excited state through Lewis acid-base adduct formation. No significant spectral changes were observed in control experiments with the tetrabutylammonium cation. Titration data with Li(+), Na(+), Mg(2+), Ca(2+), Zn(2+), Al(3+), Y(3+), and La(3+) showed that the extent of stabilization saturated at high cation concentration with magnitudes that scaled roughly with the cation charge-to-size ratio. The visible absorption spectra of D2Q was particularly informative due to the presence of two well-resolved MLCT absorption bands: (1) Ru → bpy, λmax ≈ 450 nm; and (2) Ru → dcbq, λmax ≈ 540 nm. The higher-energy band blue-shifted and the lower-energy band red-shifted upon cation addition. The PL intensity and lifetime of the excited state of B2B first increased with cation addition without significant shifts in the measured spectra, behavior attributed to a cation-induced change in the localization of the emissive excited state from bpy to dcb. The importance of excited-state localization and stabilization for solar energy conversion is discussed. PMID:27391279

  9. Nuclear Quadrupole Coupling Constants in Niobium Pentachloride and Related Compounds (II) Transition Metal Nuclei

    NASA Astrophysics Data System (ADS)

    Okubo, Noriaki

    1982-02-01

    93Nb NQR spectrum in NbCl5 has been investigated from 4.2 K to 480 K. The coupling constant shows an unusual positive temperature dependence at low temperatures. The EFG tensor is calculated with the d2sp3 octahedral bond functions. The experimental data are analysed in terms of the contributions from the σ- and π-bonds. It is shown that the positive temperature dependence can be explained by the pπ-dπ bond mechanism. The theory is also applied to the related compounds and the consistency with the analysis of the halogen coupling constants is shown.

  10. Physics of Unstable Nuclei

    NASA Astrophysics Data System (ADS)

    Khoa, Dao Tien; Egelhof, Peter; Gales, Sydney; Giai, Nguyen Van; Motobayashi, Tohru

    2008-04-01

    Studies at the RIKEN RI beam factory / T. Motobayashi -- Dilute nuclear states / M. Freer -- Studies of exotic systems using transfer reactions at GANIL / D. Beaumel et al. -- First results from the Magnex large-acceptance spectrometer / A. Cunsolo et al. -- The ICHOR project and spin-isospin physics with unstable beams / H. Sakai -- Structure and low-lying states of the [symbol]He exotic nucleus via direct reactions on proton / V. Lapoux et al. -- Shell gap below [symbol]Sn based on the excited states in [symbol]Cd and [symbol]In / M. Górska -- Heavy neutron-rich nuclei produced in the fragmentation of a [symbol]Pb beam / Zs. Podolyák et al. -- Breakup and incomplete fusion in reactions of weakly-bound nuclei / D.J. Hinde et al. -- Excited states of [symbol]B and [symbol]He and their cluster aspect / Y. Kanada-En'yo et al. -- Nuclear reactions with weakly-bound systems: the treatment of the continuum / C. H. Dasso, A. Vitturi -- Dynamic evolution of three-body decaying resonances / A. S. Jensen et al. -- Prerainbow oscillations in [symbol]He scattering from the Hoyle state of [symbol]C and alpha particle condensation / S. Ohkubo, Y. Hirabayashi -- Angular dispersion behavior in heavy ion elastic scattering / Q. Wang et al. -- Microscopic optical potential in relativistic approach / Z.Yu. Ma et al. -- Exotic nuclei studied in direct reactions at low momentum transfer - recent results and future perspectives at fair / P. Egelhof -- Isotopic temperatures and symmetry energy in spectator fragmentation / M. De Napoli et al. -- Multi-channel algebraic scattering theory and the structure of exotic compound nuclei / K. Amos et al. -- Results for the first feasibility study for the EXL project at the experimental storage ring at GSI / N. Kalantar-Nayestanaki et al. -- Coulomb excitation of ISOLDE neutron-rich beams along the Z = 28 chain / P. Van Duppen -- The gamma decay of the pygmy resonance far from stability and the GDR at finite temperature / G. Benzoni et al

  11. Nuclear Quadrupole Coupling Constants in Niobium Pentachloride and Related Compounds (I) Halogen Nuclei

    NASA Astrophysics Data System (ADS)

    Okubo, Noriaki

    1982-02-01

    35Cl NQR spectrum in NbCl5 has been investigated from 4.2 K to 480 K. The lines of about 7 MHz have larger multiplicity and show positive temperature dependence in contrast to the usual negative one for the line of about 13 MHz. The former lines are further separated into two groups having different temperature dependences. The expressions for the chlorine coupling constant are derived according to Townes-Dailey’s method on the basis of the pπ-dπ bond. The NQR data are analysed and the lines are assigned to the axial, equatorial and bridging chlorine atoms in the Nb2Cl10 dimer. The theory is applied to other related compounds.

  12. Fission Study of Actinide Nuclei Using Multi-nucleon Transfer Reactions

    NASA Astrophysics Data System (ADS)

    Nishio, Katsuhisa; Hirose, Kentaro; Léguillon, R.; Makii, Hiroyuki; Nishinaka, Ichiro; Orlandi, Riccardo; Smallcombe, James; Tsukada, Kazuaki; Chiba, Satoshi; Ohtsuki, Tsutomu; Tatsuzawa, Ryotaro; Takaki, Naoyuki

    We have developed a set up to measure fission properties of excited compound nuclei populated by multi-nucleon transfer reactions. This approach has an advantage that we can study fission of neutron-rich nuclei which cannot be accessed by particle or charged-particle capture reactions. Unique feature in our setup is that we can produce fission data for many nuclei depending on different transfer channels. Also wide excitation energy range can be covered in this set up, allowing us to measure the excitation energy dependence of the fission properties. Preliminary data obtained in the 18O + 238U reaction will be presented.

  13. The decay of hot nuclei

    SciTech Connect

    Moretto, L.G.; Wozniak, G.J.

    1988-11-01

    The formation of hot compound nuclei in intermediate-energy heavy ion reactions is discussed. The statistical decay of such compound nuclei is responsible for the abundant emission of complex fragments and high energy gamma rays. 43 refs., 23 figs.

  14. Permissible overheating of the gaseous medium in a gas-flow laser excited by fission fragments from uranium nuclei

    SciTech Connect

    Prikhod'ko, E V; Sizov, A N

    1999-09-30

    The limits on the permissible overheating of the gaseous mixtures in gas-flow lasers excited by uranium-nuclear-fission fragments are examined. The first limit is associated with the possibility of growth of a heat-removal zone near the walls and the second arises from the need to preserve the cavity stability. (active media)

  15. Quantification of multiple compounds containing heterogeneous elements in the mixture by one-dimensional nuclear magnetic resonance spectroscopy of different nuclei using a single universal concentration reference.

    PubMed

    Xu, Li; Shi, Xiaohuo; Hu, Kaifeng

    2014-12-01

    One-dimensional (1D) quantitative NMR (qNMR) is a useful tool for concentration determination due to its experimental simplicity and the direct proportionality of the integrated signal area to the number of nuclei spin. For complex mixtures, however, signal overlapping often in one-dimensional quantitative (1) H NMR (1D (1) H qNMR) spectrum limits the accurate quantification of individual compound. Here, we introduced employing joint 1D qNMR methods of different nuclei, such as (1) H and (31) P (or/and (19) F), to quantify multiple compounds in a complex mixture using a single universal concentration reference. When the concentration ratio of several compounds containing different elements in a complex mixture is of interest, the result calculated from measured intensities from 1D qNMR of different nuclei is independent of the gravimetric error from the reference. In this case, the common reference also serves as a 'quantitative bridge' among these 1D qNMR of different nuclei. Quantitative analysis of choline, phosphocholine, and glycerophosphocholine mixture is given as an example using trimethylphosphine oxide ((CH(3))(3) P(O)) as concentration reference. Compounds containing multiple elements, such as tetramethylammonium hexafluorophosphate (N(+) (CH(3))(4 PF6 (-) are proposed as the common concentration reference for (1) H, (13) C, (15) N, (31) P, and (19) F qNMR for the quantitative analysis of complex mixture containing these different elements. We anticipate that the proposed joint 1D qNMR approach using a universal concentration reference will be a valuable alternative for simultaneous quantification of multiple compounds in a complex mixture due to its accuracy and single and simple sample preparation. PMID:25298349

  16. Photoformation of Triplet Excited States and Other Oxidants in Fog Waters and Their Impact on Fog Processing of Organic Compounds

    NASA Astrophysics Data System (ADS)

    Kaur, R.; Anastasio, C.; Valsaraj, K. T.; Vempati, H. S.; Vaitilingom, M.

    2014-12-01

    Reactions in fog and cloud drops are important for a number of processes, such as formation of secondary organic aerosol (SOA), cycling of organic carbon and nitrogen, and determining the lifetimes of pollutants. The rates of these processes depend upon the steady-state concentrations of the major photooxidants, namely, hydroxyl radical (.OH), singlet molecular oxygen (1O2*) and triplet excited states of organic compounds (3C*). While there are some past measurements of .OH and 1O2* concentrations in fog and cloud drops, there are no data for the concentrations of triplet excited states. However, there is increasing evidence that triplets might be important for the processing of organics in a cloudy or foggy atmosphere. To address this question, we collected fog water samples from Davis, CA and Baton Rouge, LA, illuminated them with simulated sunlight, and measured the steady-state concentrations of .OH , 1O2* and 3C* . To understand the relative importance of these photooxidants, we also measured the photochemical loss of two added model organic compounds in the illuminated fog waters - syringol (a biomass burning phenol) and methyl jasmonate (a green leaf volatile). Our results show that triplet excited states can play a major role in oxidizing the model compounds, typically accounting for 30 - 90% of the loss of both model compounds. Given that atmospheric triplets are relatively less understood, our results highlight the importance of deeper investigation into their nature.

  17. Ground and excited states of doubly open-shell nuclei from ab initio valence-space Hamiltonians

    NASA Astrophysics Data System (ADS)

    Stroberg, S. R.; Hergert, H.; Holt, J. D.; Bogner, S. K.; Schwenk, A.

    2016-05-01

    We present ab initio predictions for ground and excited states of doubly open-shell fluorine and neon isotopes based on chiral two- and three-nucleon interactions. We use the in-medium similarity renormalization group to derive mass-dependent s d valence-space Hamiltonians. The experimental ground-state energies are reproduced through neutron number N =14 , beyond which a new targeted normal-ordering procedure improves agreement with data and large-space multireference calculations. For spectroscopy, we focus on neutron-rich F-2623 and Ne-2624 isotopes near N =14 ,16 magic numbers. In all cases we find agreement with experiment and established phenomenology. Moreover, yrast states are well described in 20Ne and 24Mg, providing a path toward an ab initio description of deformation in the medium-mass region.

  18. Resonance phenomena: From compound nucleus decay to proton radioactivity

    NASA Astrophysics Data System (ADS)

    Charity, R. J.

    2016-03-01

    The role of resonances in exotic nuclei is investigated. This encompasses one and two nucleon emitters for ground-state nuclei beyond the drip lines to compound nuclei formed at higher excitation energies which, in some cases, can decay to produce these ground-state emitters. The role of barrier penetration and configuration mixing are both considered in explaining the long lifetimes observed in narrow resonances. Finally, two experimental techniques for studying exotic resonances are presented.

  19. Characterization of the multifragment decay channel in highly excited nuclei. Progress report, March 15, 1992--September 14, 1993

    SciTech Connect

    de Souza, R.T.

    1992-10-01

    Characteristics of multifragment decay in heavy-ion induced reactions at intermediate energies are explored. Evolution of the timescale for emission of intermediate mass fragments (IMF: 3{le}Z{le}20) is investigated. Fragments associated with central collisions in the reactions {sup 36}Ar + {sup 197}Au at E/A = 50, 80, and 110 MeV are emitted on an extremely fast timescale, {tau} {le} 75 fm/c, comparable to the transit time of the projectile past the target nucleus. With increasing incident energy, mean fragment emission times decrease, consistent with statistical decay from highly excited systems or fast dynamical processes. To examine the importance of expansion effects in multifragmentation, the transverse kinetic energy of fragments was investigated. Evidence for expansion effects in the system {sup 36}Ar + {sup 197}Au at E/A = 50, 80, and 110 MeV was indicated by the charge dependence of the mean isotropic kinetic energy. At the highest incident energy the data suggest the onset of volume emission. Construction and performance of low-threshold high-resolution detector telescopes is discussed. Three-body Coulomb trajectory calculations are being used to probe kinematical correlations associated with neck emission of IMFs during fission. Initial design and testing of position sensitive parallel plate avalanche counters for upcoming ternary fission experiments is discussed.

  20. Formation of superheavy nuclei in cold fusion reactions

    SciTech Connect

    Feng Zhaoqing; Jin Genming; Li Junqing; Scheid, Werner

    2007-10-15

    Within the concept of the dinuclear system (DNS), a dynamical model is proposed for describing the formation of superheavy nuclei in complete fusion reactions by incorporating the coupling of the relative motion to the nucleon transfer process. The capture of two heavy colliding nuclei, the formation of the compound nucleus, and the de-excitation process are calculated by using an empirical coupled channel model, solving a master equation numerically and applying statistical theory, respectively. Evaporation residue excitation functions in cold fusion reactions are investigated systematically and compared with available experimental data. Maximal production cross sections of superheavy nuclei in cold fusion reactions with stable neutron-rich projectiles are obtained. Isotopic trends in the production of the superheavy elements Z=110, 112, 114, 116, 118, and 120 are analyzed systematically. Optimal combinations and the corresponding excitation energies are proposed.

  1. Evolution of the mixed-symmetry 2{sup+}{sub 1,ms} quadrupole-photon excitation from spherical to {gamma}-soft Xe nuclei.

    SciTech Connect

    Coquard, L.; Pietralla, N.; Rainovski, G.; Ahn, T.; Bettermann, L.; Carpenter, M. P.; Janssens, R.V. F.; Leske, J.; Lister, C. J.; Moller, O.; Rother, W.; Werner, V.; Zhu, S.

    2010-08-23

    Low-lying collective states of {sup 130,132}Xe have been investigated by {gamma}-ray spectroscopy following {sup 12}C(Xe,Xe*){sup 12}C projectile Coulomb excitation. The one-phonon 2{sub 1,ms}{sup +} states have been identified: the 2{sub 4}{sup +} state at 2150 keV with B(M1;2{sub 4}{sup +} {yields} 2{sub 1}{sup +})=0.15(4){mu}{sub {mu}}{sup N} in {sup 130}Xe and the 2{sub 3}{sup +} state at 1985 keV with B(M1;2{sub 3}{sup +} {yields} 2{sub 1}{sup +})=0.22(6){mu}{sub N}{sup 2} in {sup 132}Xe. The evolution of the one-phonon 2{sub 1,ms}{sup +} states in the even-even stable xenon isotopic chain from the vibrators near N=82 to the {gamma}-soft nuclei toward midshell is discussed.

  2. Strong M1 components in 3{sub i}{sup -}->3{sub 1}{sup -} transitions in nearly spherical nuclei: Evidence for isovector-octupole excitations

    SciTech Connect

    Scheck, M.; Butler, P. A.; Fransen, C.; Werner, V.; Yates, S. W.

    2010-06-15

    An evaluation of data obtained in (n,n{sup '}gamma) experiments reveals strong M1 3{sub i}{sup -}->3{sub 1}{sup -} transitions in nuclei near the N=50 ({sup 92}Zr, {sup 94}Mo, and {sup 96}Mo), Z=50 ({sup 112}Cd and {sup 114}Cd), and N=82 ({sup 144}Nd) shell closures. The observed <3{sub 1}{sup -}||M1||3{sub i}{sup -}> matrix elements scale with the <2{sub 1}{sup +}||M1||2{sub ms}{sup +}> matrix elements connecting the mixed-symmetric and symmetric quadrupole excitations. In accordance with a picture of a mixed two-component quantum system, the energy difference between the initial 3{sub i}{sup -} state and the 3{sub 1}{sup -} octupole phonon is proportional to the |<3{sub 1}{sup -}||E3||0{sub gs}{sup +}>| matrix element. The possibility of assigning the 3{sup -} states of interest as octupole isovector states is discussed.

  3. Non-coplanar compact configurations of nuclei and non-compound-nucleus contribution in the fusion cross section of the 12C+93Nb reaction

    NASA Astrophysics Data System (ADS)

    Chopra, Sahila; Hemdeep, Kaur, Arshdeep; Gupta, Raj K.

    2016-02-01

    Background: In our earlier study of the 12C+93Nb→*105Ag reaction at three near- and below-barrier energies (Ec .m .=41.097 , 47.828, and 54.205 MeV), using the dynamical cluster-decay model (DCM) with various nuclear interaction potentials (the Blocki et al. pocket formula and others derived from the Skyrme energy density formalism) for compact, coplanar (Φc=00 ) nuclei, we found a large non-compound-nucleus (nCN) contribution in the measured fusion cross section of this reaction. Purpose: In the present work, we look for the effect of using non-coplanar, compact configurations (Φc≠00 ), in the Blocki et al. pocket formula of the nuclear proximity potential, on the non-compound-nucleus (nCN) contribution, using the DCM. Methods: Allowing the Φ degree of freedom in the DCM formalism, we calculate the compound-nucleus (CN) and nCN cross sections. The only parameter of the DCM is the neck-length parameter Δ R , which also fits the empirically determined nCN cross section nearly exactly, under the assumption of considering it like a quasifission process where the fragment preformation factor P0=1 . Results: With the Φ degree of freedom included, at the higher two energies the nCN cross section gets enhanced, and hence the pure CN cross section is decreased, since the calculated (total) fusion cross section is fitted to experimental data. The parameter Δ R for the nCN contribution is smaller, and hence the reaction time larger, than for the CN decay process. Also, the contributing angular momentum ℓmax value increases in going from Φc=00 to Φc≠00 for both the CN and nCN processes. The intermediate mass fragments (IMFs), measured up to mass 13 in this reaction, are shown extended up to mass 16, and the fusion-fission (f f ) region is identified as A /2 ±16 , the same as for the Φc=00 case. Conclusions: As a result of enhanced nCN cross section due to Φc≠00 , the CN fusion probability PCN for *105Ag changes its behavior from an increasing to a

  4. Electronic excitation transport in photosynthesis and crystal and molecular structures of porphyrin compounds

    SciTech Connect

    Yang, Shumei.

    1991-04-22

    The excitation energy transfer in three photosynthetic organism samples, Bacteriochlorophyll a-protein from Prosthecochloris aestuarii, and enriched photosystem I particles from spinach chloroplasts, have been investigated by pump-probe ultrafast spectroscopy. The isotropic photobleaching profiles were best described by two exponential decay components in one Bchl a-protein complex, and three exponential decay components in another. The experimental results from the three samples show that nonrandom chromophore orientations exist and Sauer's pebble mosaic'' model is an appropriate one for excitation transfer in these samples. The polarized pump-probe transients have been analyzed in terms of an exciton hopping model that incorporates the known geometry of the Bchl a-protein. The crystal and molecular structures of four metalloporphyrins have been determined by X-ray diffraction and molecular mechanics. 207 refs., 44 figs., 15 tabs.

  5. Radiations from hot nuclei

    NASA Technical Reports Server (NTRS)

    Malik, F. Bary

    1993-01-01

    The investigation indicates that nuclei with excitation energy of a few hundred MeV to BeV are more likely to radiate hot nuclear clusters than neutrons. These daughter clusters could, furthermore, de-excite emitting other hot nuclei, and the chain continues until these nuclei cool off sufficiently to evaporate primarily neutrons. A few GeV excited nuclei could radiate elementary particles preferentially over neutrons. Impact of space radiation with materials (for example, spacecraft) produces highly excited nuclei which cool down emitting electromagnetic and particle radiations. At a few MeV excitation energy, neutron emission becomes more dominant than gamma-ray emission and one often attributes the cooling to take place by successive neutron decay. However, a recent experiment studying the cooling process of 396 MeV excited Hg-190 casts some doubt on this thinking, and the purpose of this investigation is to explore the possibility of other types of nuclear emission which might out-compete with neutron evaporation.

  6. Origin of longitudinal spin excitations in iron-pnictide parent compounds

    NASA Astrophysics Data System (ADS)

    Fidrysiak, Maciej

    2016-02-01

    We investigate longitudinal spin excitations (LSEs) as a probe of microscopic origin of magnetic ordering in parent pnictides BaFe2As2 and NaFeAs. Currently adopted interpretation of LSEs as bottom of particle-hole continuum points unambiguously toward itinerant-electron magnetism, but is difficult to reconcile with available optical measurements. We study the possibility that the LSEs originate from multi-magnon processes which are not energetically constrained by optical spectroscopy and do not sharply distinguish between local-moment and itinerant scenarios. Two mechanisms, capable of enhancing multi-magnon continuum to the level indicated by neutron scattering experiments, are proposed. The first emphasizes itinerant electrons and is based on electronic transitions between magnetically split bands, while the other relies on purely spin fluctuations close to a magnetic quantum phase transition. Electronic excitations enhance multi-magnon contribution to LSEs for small Fermi surface taking part in the SDW instability, but are insufficient to account for measured intensities. The correct order of LSEs, on the other hand, can be reproduced by the spin fluctuation mechanism for a reasonable set of parameters.

  7. Magnon excitation and temperature dependent transport properties in magnetic tunnel junctions with Heusler compound electrodes

    NASA Astrophysics Data System (ADS)

    Drewello, Volker; Ebke, Daniel; Schäfers, Markus; Kugler, Zoë; Reiss, Günter; Thomas, Andy

    2012-04-01

    Magnetic tunnel junctions were prepared with the Heusler compounds Co2FeAl, Co2FeSi, and Co2MnSi as the soft magnetic electrode. The Co2MnSi electrodes had a multilayer design that used either the Co2FeAl or the Co2FeSi compound as a buffer material. Pinned Co-Fe was used as the hard reference electrode. The electronic transport characteristics were analyzed by tunneling spectroscopy. The dependence of sample properties on the buffer material was of interest, especially the gap in the minority density of states of the Heusler electrode. The temperature dependence of the transport properties was also investigated.

  8. Quartet excited halogen atoms produced in the electron pulse irradiation of rare gases containing halogenated compounds

    NASA Astrophysics Data System (ADS)

    Kuramasu, T.; Ohyama, H.; Yoshikawa, S.; Terazawa, N.; Ishikawa, Y.; Arai, S.

    1995-07-01

    Quartet excited halogen atoms F*(2p4 3s,4PJ), Cl*(3p4 4s,4PJ), Br*(4p4 5s,4PJ), and I*(5p4 6s,4PJ), where the J's are 5/2, 3/2, and 1/2, were found to be produced in the electron pulse irradiation of Ne or Ar containing one of SF6, CCl4, CClF3, CBrF3, CBr2F2, and CF3I. The population distribution ratios at the stage of production were 1.0(J=5/2):0.41(J=3/2):0.06(J=1/2) for F* in Ne containing SF6, 1.0(J=5/2):0.27(J=3/2):0.14(J=1/2) for Cl* in Ne containing CCl4, 1.0(J=5/2):0.29(J=3/2):0.2-0.3(J=1/2) for Br* in Ne containing CBr2F2, and 1.0(J=5/2):0.13(J=3/2):0.54(J=1/2) for I* in Ar containing CF3I. The observed ratios considerably differ from those calculated from the Boltzmann distribution law. F*(4P5/2), F*(4P3/2), and Cl*(4P5/2) are mainly produced by the reactions of lowest triplet excited diatomic molecules of neon with SF6 and CCl4. Cl*(4P3/2) and Cl*(4P1/2) are produced in a rapid process and deactivated into lower Cl*(4P5/2). Several reaction channels probably contribute to the formation of Br*(4PJ) and I*(4PJ). Rate constants for reactions of triplet excited diatomic molecules of neon or argon with these parent molecules were determined from observed absorption decay curves for Ne2* or Ar2* in the presence of parent molecules.

  9. Photoreactivity of biologically active compounds. XIX: excited states and free radicals from the antimalarial drug primaquine.

    PubMed

    Kristensen, Solveig; Edge, Ruth; Tønnesen, Hanne Hjorth; Bisby, Roger Hugh; Navaratnam, Suppiah

    2009-03-01

    The formation and reactivity of excited states and free radicals from primaquine, a drug used in the treatment of malaria, was studied in order to evaluate the primary photochemical reaction mechanisms. The excited primaquine triplet was not detected, but is likely to be formed with a short lifetime (<50 ns) and with a triplet energy <250 kJ/mol as the drug is an efficient quencher of the fenbufen triplet and the biphenyl triplet, and forms (1)O(2) by laser flash photolysis ((PQ)Phi(Delta)=0.025). Primaquine (PQ) exists as the monocation (PQH(+)) in aqueous solution at physiological pH. PQH(+) photoionises by a biphotonic process and also forms the monoprotonated cation radical (PQH(2+)*) by one electron oxidation by HO* (k(q)=6.6 x 10(9) M(-1) s(-1)) and Br*(2)(-) (k(q)=4.7 x 10(9) M(-1) s(-1)) at physiological pH, detected as a long-lived transient decaying essentially by a second order process (k(2)=7.4 x 10(8) M(-1) s(-1)). PQH(2+)* is scavenged by O(2), although at a limited rate (k(q)=1.0 x 10(6) M(-1) s(-1)). The reduction potential (E degrees) of PQH(2+)*/PQH(+) is < +1015 mV, as measured versus tryptophan (TRP*/TRPH). Primaquine also forms PQH(2+)* at pH 2.4, by one electron oxidation by Br*(2)(-) and proton loss (k(q)=2.7 x 10(9) M(-1) s(-1)). The non-protonated cation radical (PQ(+)*) is formed during one electron oxidation with Br*(2)(-) at alkaline conditions (k(q)=4.2 x 10(9) M(-1) s(-1) at pH 10.8). The estimated pK(a)-value of PQH(2+)*/PQ(+)* is pK(a) approximately 7-8. Primaquine is not a scavenger of O*(2)(-) at physiological pH. Thus self-sensitization by O*(2)(-) is eliminated as a degradation pathway in the photochemical reactions. Impurities in the raw material and photochemical degradation products initiate photosensitized degradation of primaquine in deuterium oxide, prevented by addition of the (1)O(2) quencher sodium azide. Photosensitized degradation by formation of (1)O(2) is thus important for the initial photochemical decomposition of

  10. Asymmetrical fission and statistical emission of complex fragments from the highly excited {sup 47}V compound nucleus

    SciTech Connect

    Beck, C.; Djerroud, B.; Haas, F.; Freeman, R.M.; Hachem, A.; Heusch, B.; Morsad, A.; Vuillet-A-Crilles, M.; Youlal, M.; Abe, Y.; Dayras, R.; Wieleczko, J.P.; Legrain, R.; Pollaco, E.; Ray, A.; Shapira, D.; Campo, J.G.D.; Kim, H.J.; Cavallaro, S.; De Fillippo, E.; Lanzano, G.; Pagano, A.; Sperduto, M.L.; Matsuse, T.; Sanders, S.J.

    1991-12-31

    The properties of the fully damped (deep-inelastic and orbiting) and fusion (evaporation and fission) processes have been investigated in three entrance channels leading to the same {sup 47} V compound nucleus at high excitation energies. No entrance channel effect has been observed in either the evaporation residue or the fission-like yields in contrast to the {sup 28}Si + {sup 12}C and {sup 24}Mg + {sup 16}O reactions in which the orbiting process still persists. The asymmetrical elemental distributions of the fully energy relaxed fragments are well described by fusion-fission models based respectively on the scission point and saddle point pictures. Finally a general discussion of the competition between orbiting and fusion-fission mechanisms in light heavy-ion reactions is presented in the framework of their calculated available number of open channels.

  11. The TDPAC study of the hyperfine interactions at 111Cd nuclei in RAl 3 compounds synthesized under high pressure

    NASA Astrophysics Data System (ADS)

    Tsvyashchenko, A. V.; Fomicheva, L. N.; Brudanin, V. B.; Kochetov, O. I.; Salamatin, A. V.; Velichkov, A.; Wiertel, M.; Budzynski, M.; Sorokin, A. A.; Ryasny, G. K.; Komissarova, B. A.

    2007-06-01

    The time-differential perturbed angular correlations technique (TDPAC) has been employed for measuring the parameters of hyperfine interactions in earlier known RAl 3 compounds, synthesized at high pressure (8 GPa) and high temperature, where R = La, Ce, Sm, Gd, Tb, Dy, Ho, Er, Yb and Lu. The 111Cd( 111In) radioactive atom was used as a probe nucleus. The X-ray method has revealed that with the increase in the atomic number of a rare-earth element R, the obtained RAl 3 high-pressure phases crystallize, respectively, into orthorhombic, hexagonal and cubic structures. It has been found that in the compounds containing R=La, Ce, Sm and Gd, a deviation from earlier known structural types and the formation of new ones is observed, which is associated with the change of the stoichiometric composition of the said compounds. The results of the PAC measurements have confirmed the deviation from the predetermined stoichiometric composition 1R:3Al for the compounds LaAl 3, CeAl 3, SmAl 3 and GdAl 3 and have verified the RAl 3 stoichiometric structure for the other high-pressure phases obtained in this work.

  12. Effect of organic compounds on cloud condensation nuclei (CCN) activity of sea spray aerosol produced by bubble bursting

    NASA Astrophysics Data System (ADS)

    Moore, Meagan J. K.; Furutani, Hiroshi; Roberts, Gregory C.; Moffet, Ryan C.; Gilles, Mary K.; Palenik, Brian; Prather, Kimberly A.

    2011-12-01

    The ocean comprises over 70% of the surface of the earth and thus sea spray aerosols generated by wave processes represent a critical component of our climate system. The manner in which different complex oceanic mixtures of organic species and inorganic salts are distributed between individual particles in sea spray directly determines which particles will effectively form cloud nuclei. Controlled laboratory experiments were undertaken to better understand the full range of particle properties produced by bubbling solutions composed of simplistic model organic species, oleic acid and sodium dodecyl sulfate (SDS), mixed with NaCl to more complex artificial seawater mixed with complex organic mixtures produced by common oceanic microorganisms. Simple mixtures of NaCl and oleic acid or SDS had a significant effect on CCN activity, even in relatively small amounts. However, an artificial seawater (ASW) solution containing microorganisms, the common cyanobacteria ( Synechococcus) and DMS-producing green algae ( Ostreococcus), produced particles containing ˜34 times more carbon than the particles produced from pure ASW, yet no significant change was observed in the overall CCN activity. We hypothesize that these microorganisms produce diverse mixtures of organic species with a wide range of properties that produced offsetting effects, leading to no net change in the overall average measured hygroscopicity of the collection of sea spray particles. Based on these observations, changes in CCN activity due to "bloom" conditions would be predicted to lead to small changes in the average CCN activity, and thus have a negligible impact on cloud formation. However, each sea spray particle will contain a broad spectrum of different species, and thus further studies are needed of the CCN activity of individual sea spray particles and biological processes under a wide range of controllable conditions.

  13. Transfer involving deformed nuclei

    SciTech Connect

    Rasmussen, J.O.; Guidry, M.W.; Canto, L.F.

    1985-03-01

    Results are reviewed of 1- and 2-neutron transfer reactions at near-barrier energies for deformed nuclei. Rotational angular momentum and excitation patterns are examined. A strong tendency to populating high spin states within a few MeV of the yrast line is noted, and it is interpreted as preferential transfer to rotation-aligned states. 16 refs., 12 figs.

  14. New Experimental Insight into the Nature of Metal-Metal Bonds in Digallium Compounds: J Coupling between Quadrupolar Nuclei.

    PubMed

    Kobera, Libor; Southern, Scott A; Rao, Gyandshwar Kumar; Richeson, Darrin S; Bryce, David L

    2016-07-01

    Multiple bonding between atoms is of ongoing fundamental and applied interest. Here, we report a multinuclear ((1) H, (13) C, and (71) Ga) solid-state magnetic resonance spectroscopic study of digallium compounds which have been proposed, albeit somewhat controversially, to contain single, double, and triple Ga-Ga bonds. Of particular relevance to the nature of these bonds, we have carried out two-dimensional (71) Ga J/D-resolved NMR experiments which provide a direct measurement of J((71) Ga,(71) Ga) spin-spin coupling constants across the gallium-gallium bonds. When placed in the context of clear-cut experimental data for analogous singly, doubly, and triply bonded carbon spin pairs or boron spin pairs, the (71) Ga NMR data clearly support the notion of a different bonding paradigm in the gallium systems. Our findings are consistent with an increasing role across the purported gallane-gallene-gallyne series for classical and/or slipped π-type bonding orbitals. PMID:27276691

  15. Dirac-Hartree-Bogoliubov calculation for spherical and deformed hot nuclei: Temperature dependence of the pairing energy and gaps, nuclear deformation, nuclear radii, excitation energy, and entropy

    NASA Astrophysics Data System (ADS)

    Lisboa, R.; Malheiro, M.; Carlson, B. V.

    2016-02-01

    Background: Unbound single-particle states become important in determining the properties of a hot nucleus as its temperature increases. We present relativistic mean field (RMF) for hot nuclei considering not only the self-consistent temperature and density dependence of the self-consistent relativistic mean fields but also the vapor phase that takes into account the unbound nucleon states. Purpose: The temperature dependence of the pairing gaps, nuclear deformation, radii, binding energies, entropy, and caloric curves of spherical and deformed nuclei are obtained in self-consistent RMF calculations up to the limit of existence of the nucleus. Method: We perform Dirac-Hartree-Bogoliubov (DHB) calculations for hot nuclei using a zero-range approximation to the relativistic pairing interaction to calculate proton-proton and neutron-neutron pairing energies and gaps. A vapor subtraction procedure is used to account for unbound states and to remove long range Coulomb repulsion between the hot nucleus and the gas as well as the contribution of the external nucleon gas. Results: We show that p -p and n -n pairing gaps in the S10 channel vanish for low critical temperatures in the range Tcp≈0.6 -1.1 MeV for spherical nuclei such as 90Zr, 124Sn, and 140Ce and for both deformed nuclei 150Sm and 168Er. We found that superconducting phase transition occurs at Tcp=1.03 Δp p(0 ) for 90Zr, Tcp=1.16 Δp p(0 ) for 140Ce, Tcp=0.92 Δp p(0 ) for 150Sm, and Tcp=0.97 Δp p(0 ) for 168Er. The superfluidity phase transition occurs at Tcp=0.72 Δn n(0 ) for 124Sn, Tcp=1.22 Δn n(0 ) for 150Sm, and Tcp=1.13 Δn n(0 ) for 168Er. Thus, the nuclear superfluidity phase—at least for this channel—can only survive at very low nuclear temperatures and this phase transition (when the neutron gap vanishes) always occurs before the superconducting one, where the proton gap is zero. For deformed nuclei the nuclear deformation disappear at temperatures of about Tcs=2.0 -4.0 MeV , well above the

  16. Comparative effects of sulfhydryl compounds on target organellae, nuclei and mitochondria, of hydroxylated fullerene-induced cytotoxicity in isolated rat hepatocytes.

    PubMed

    Nakagawa, Yoshio; Inomata, Akiko; Ogata, Akio; Nakae, Dai

    2015-12-01

    DNA damage and cytotoxicity induced by a hydroxylated fullerene [C60 (OH)24 ], which is a spherical nanomaterial and/or a water-soluble fullerene derivative, and their protection by sulfhydryl compounds were studied in freshly isolated rat hepatocytes. The exposure of hepatocytes to C60 (OH)24 at a concentration of 50 μM caused time (0 to 3 h)-dependent cell death accompanied by the formation of cell surface blebs, the loss of cellular levels of ATP and reduced glutathione, accumulation of glutathione disulfide, and induction of DNA fragmentation assayed using alkali single-cell agarose-gel electrophoresis. C60 (OH)24 -induced cytotoxicity was effectively prevented by pretreatment with sulfhydryl compounds. N-acetyl-L-cysteine (NAC), L-cysteine and L-methionine, at a concentration of 2.5 mM, ameliorated cell death, accompanied by a decrease in cellular ATP levels, formation of cell surface blebs, induction of reactive oxygen species (ROS) and loss of mitochondrial membrane potential caused by C60 (OH)24 . In addition, DNA fragmentation caused by C60 (OH)24 was also inhibited by NAC, whereas an antioxidant ascorbic acid did not affect C60 (OH)24 -induced cell death and DNA damage in rat hepatocytes. Taken collectively, these results indicate that incubation of rat hepatocytes with C60 (OH)24 elicits DNA damage, suggesting that nuclei as well as mitochondria are target sites of the hydroxylated fullerene; and induction of DNA damage and oxidative stress is ameliorated by an increase in cellular GSH levels, suggesting that the onset of toxic effects may be partially attributable to a thiol redox-state imbalance caused by C60 (OH)24 . PMID:25809591

  17. Nuclear spectroscopy above isomers in {sub 67}{sup 148}Ho{sub 81} and {sub 67}{sup 149}Ho{sub 82} nuclei: Search for core-excited states in {sup 149}Ho

    SciTech Connect

    Kownacki, J.; Napiorkowski, P. J.; Zielinska, M.; Kordyasz, A.; Srebrny, J.; Droste, Ch.; Morek, T.; Grodner, E.; Ruchowska, E.; Korman, A.; Czarnacki, W.; Kisielinski, M.; Kowalczyk, M.; Wrzosek-Lipska, K.; Hadynska-KlePk, K.; Mierzejewski, J.; Lieder, R. M.; Perkowski, J.; Andrzejewski, J.; Krol, A.

    2010-04-15

    The excited states of {sup 148}Ho and {sup 149}Ho isotopes are studied using gamma-ray and electron spectroscopy in off-beam and in-beam modes following {sup 112,114}Sn({sup 40}Ar,xnyp) reactions. Experiments include measurements of single gamma-rays and conversion electron spectra as well as gamma-gamma, electron-gamma, gamma-t, and gamma-gamma-t coincidences with the use of the OSIRIS-II 12-HPGe array and conversion electron spectrometer. Based on the present results, the level schemes of {sup 148}Ho and {sup 149}Ho are revised and significantly extended, up to about 4 and 5 MeV of excitation energy, respectively. Spin and parity of 5{sup -} are assigned to the 9.59-s isomer in {sup 148}Ho based on conversion electron results. Previously unobserved gamma rays feeding the 10{sup +} isomer in {sup 148}Ho and the 27/2{sup -} isomer in {sup 149}Ho nuclei are proposed. Shell-model calculations are performed. Possible core-excited states in {sup 149}Ho are discussed.

  18. Level densities of heaviest nuclei

    NASA Astrophysics Data System (ADS)

    Bezbakh, A. N.; Shneidman, T. M.; Adamian, G. G.; Antonenko, N. V.

    2014-06-01

    The intrinsic level densities of superheavy nuclei in the α-decay chains of 296,298,300120 are calculated using the single-particle spectra obtained with the modified two-center shell model. The role of the shell and pairing effects on the level density as well as their quenching with excitation energy are studied. The extracted level density parameter is expressed as a function of mass number, ground-state shell correction, and excitation energy. The results are compared with the phenomenological values of level density parameters used to calculate the survival of excited heavy nuclei.

  19. Excitation-Photon-Energy Selectivity of Photoconversions in Halogen-Bridged Pd-Chain Compounds: Mott Insulator to Metal or Charge-Density-Wave State

    NASA Astrophysics Data System (ADS)

    Matsuzaki, H.; Iwata, M.; Miyamoto, T.; Terashige, T.; Iwano, K.; Takaishi, S.; Takamura, M.; Kumagai, S.; Yamashita, M.; Takahashi, R.; Wakabayashi, Y.; Okamoto, H.

    2014-08-01

    Ultrafast photoinduced transitions of a one-dimensional Mott insulator into two distinct electronic phases, metal and charge-density-wave (CDW) state, were achieved in a bromine-bridged Pd-chain compound [Pd(en)2Br](C5-Y)2H2O (en =ethylenediamine and C5-Y=dialkylsulfosuccinate), by selecting the photon energy of a femtosecond excitation pulse. For the resonant excitation of the Mott-gap transition, excitonic states are generated and converted to one-dimensional CDW domains. For the higher-energy excitation, free electron and hole carriers are produced, giving rise to a transition of the Mott insulator to a metal. Such selectivity in photoconversions by the choice of initial photoexcited states opens a new possibility for the developments of advanced optical switching and memory functions.

  20. Quadrupolar transients, cosine correlation functions, and two-dimensional exchange spectra of non-selectively excited spin-3/2 nuclei: A 7Li NMR study of the superionic conductor lithium indium phosphate

    NASA Astrophysics Data System (ADS)

    Storek, M.; Böhmer, R.

    2015-11-01

    Cos-cos stimulated echoes of non-selectively excited spin-3/2 nuclei were not exploited in studies of slow motional processes in solids and solid-like samples, so far. Based on a theoretical analysis of the quadrupolar transients which hitherto obviously precluded the application of such echoes, their utility is demonstrated for the example of 7Li NMR on the polycrystalline fast ion conductor lithium indium phosphate. Quadrupolar transients can adversely affect the shape of two- and three-pulse echo spectra and strategies are successfully tested that mitigate their impact. Furthermore, by means of suitably adapted cos-cos echo sequences an effective suppression of central-line contributions to the NMR spectra is achieved. By combining cos-cos and sin-sin datasets static two-dimensional exchange spectra were recorded that display quadrupolarly modulated off-diagonal intensity indicative of ionic motion.

  1. Fission barriers for Po nuclei produced in complete fusion reactions with heavy ions

    SciTech Connect

    Sagaidak, R. N.; Andreyev, A. N.

    2009-05-15

    Evaporation residues and fission excitation functions obtained in complete fusion reactions leading to Po compound nuclei have been analyzed in the framework of the standard statistical model. Macroscopic fission barriers deduced from the cross-section data analysis are compared with the predictions of various theoretical models and available data. A drop in the Po barriers with the decrease in a neutron number was found, which is stronger than predicted by any theory. The presence of entrance channel effects and collective excitations in the compound nucleus decay is considered as a possible reason for the barrier reduction.

  2. Statistical properties of excited nuclei in the mass range 47 Less-Than-Or-Slanted-Equal-To A Less-Than-Or-Slanted-Equal-To 59

    SciTech Connect

    Zhuravlev, B. V. Lychagin, A. A. Titarenko, N. N.; Demenkov, V. G.; Trykova, V. I.

    2012-09-15

    Level densities and their energy dependences for nuclei in the mass range of 47 {<=} A {<=} 59 were determined from the results obtained by measuring neutron-evaporation spectra in respective (p, n) reactions. The spectra of neutrons originating from the (p, n) reactions on {sup 47}Ti, {sup 48}Ti, {sup 49}Ti, {sup 53}Cr, {sup 54}Cr, {sup 57}Fe, and {sup 59}Co nuclei were measured in the proton-energy range of 7-11 MeV. These measurements were performed with the aid of a fast-neutron spectrometer by the time-of-flight method over the base of the EGP-15 pulsed tandem accelerator installed at the Institute for Physics and Power Engineering (Obninsk, Russia). A high resolution of the spectrometer and its stability in the time of flight made it possible to identify reliably discrete low-lying levels along with the continuum part of neutron spectra. Our measured data were analyzed within the statistical equilibrium and preequilibrium models of nuclear reactions. The respective calculations were performed with the aid of the Hauser-Feshbach formalismof statistical theory supplemented with the generalized model of a superfluid nucleus, the back-shifted Fermi gas model, and the Gilbert-Cameron composite formula for nuclear level densities. Nuclear level densities for {sup 47}V, {sup 48}V, {sup 49}V, {sup 53}Mn, {sup 54}Mn, {sup 57}Co, and {sup 59}Ni and their energy dependences were determined. The results are discussed and compared with available experimental data and with recommendations of model-based systematics.

  3. Photoresponse of 60Ni below 10-MeV excitation energy: Evolution of dipole resonances in fp-shell nuclei near N=Z

    NASA Astrophysics Data System (ADS)

    Scheck, M.; Ponomarev, V. Yu.; Fritzsche, M.; Joubert, J.; Aumann, T.; Beller, J.; Isaak, J.; Kelley, J. H.; Kwan, E.; Pietralla, N.; Raut, R.; Romig, C.; Rusev, G.; Savran, D.; Schorrenberger, L.; Sonnabend, K.; Tonchev, A. P.; Tornow, W.; Weller, H. R.; Zilges, A.; Zweidinger, M.

    2013-10-01

    Background: Within the last decade, below the giant dipole resonance the existence of a concentration of additional electric dipole strength has been established. This accumulation of low-lying E1 strength is commonly referred to as pygmy dipole resonance (PDR).Purpose: The photoresponse of 60Ni has been investigated experimentally and theoretically to test the evolution of the PDR in a nucleus with only a small neutron excess. Furthermore, the isoscalar and isovector M1 resonances were investigated.Method: Spin-1 states were excited by exploiting the (γ,γ') nuclear resonance fluorescence technique with unpolarized continuous bremsstrahlung as well as with fully linearly polarized, quasimonochromatic, Compton-backscattered laser photons in the entrance channel of the reaction.Results: Up to 10 MeV a detailed picture of J=1 levels was obtained. For the preponderant number of the individual levels spin and parity were firmly assigned. Furthermore, branching ratios, transition widths, and reduced B(E1) or B(M1) excitation probability were calculated from the measured scattering cross sections. A comparison with theoretical results obtained within the quasiparticle phonon model allows an insight into the microscopic structure of the observed states.Conclusions: Below 10 MeV the directly observed E1 strength [∑B(E1)↑=(153.8±9.5) e2(fm)2] exhausts 0.5% of the Thomas-Reiche-Kuhn sum rule. This value increases to 0.8% of the sum rule [∑B(E1)↑=(250.9±31.1) e2(fm)2] when indirectly observed branches to lower-lying levels are considered. Two accumulations of M1 excited spin-1 states near 8 and 9 MeV excitation energy are identified as isoscalar and isovector M1 resonances dominated by proton and neutron f7/2→f5/2 spin-flip excitations. The B(M1)↑ strength of these structures accumulates to 3.94(27)μN2.

  4. Magnetic excitations in the S =1/2 antiferromagnetic-ferromagnetic chain compound BaCu2V2O8 at zero and finite temperature

    NASA Astrophysics Data System (ADS)

    Klyushina, E. S.; Tiegel, A. C.; Fauseweh, B.; Islam, A. T. M. N.; Park, J. T.; Klemke, B.; Honecker, A.; Uhrig, G. S.; Manmana, S. R.; Lake, B.

    2016-06-01

    Unlike most quantum systems which rapidly become incoherent as temperature is raised, strong correlations persist at elevated temperatures in S =1/2 dimer magnets, as revealed by the unusual asymmetric line shape of their excitations at finite temperatures. Here, we quantitatively explore and parametrize the strongly correlated magnetic excitations at finite temperatures using high-resolution inelastic neutron scattering of the model compound BaCu2V2O8 which we show to be an alternating antiferromagnetic-ferromagnetic spin -1/2 chain. Comparison to state of the art computational techniques shows excellent agreement over a wide temperature range. Our findings hence demonstrate the possibility to quantitatively predict coherent behavior at elevated temperatures in quantum magnets.

  5. Study of near-stability nuclei populated as fission fragments in heavy-ion fusion reactions

    SciTech Connect

    Fotiadis, Nikolaos; Nelson, Ronald O; Devlin, Matthew; Cizewski, Jolie A; Krucken, Reiner; Clark, R M; Fallon, Paul; Lee, I Yang; Macchiavelli, Agusto O; Becker, John A; Younes, Walid

    2010-01-01

    Examples are presented to illustrate the power of prompt {gamma}-ray spectroscopy of fission fragments from compound nuclei with A {approx} 200 formed in fusion-evaporation reactions in experiments using the Gammasphere Ge-detector array. Complementary methods, such as Coulomb excitation and deep-inelastic processes, are also discussed. In other cases (n, xn{gamma}) reactions on stable isotopes have been used to establish neutron excitation functions for {gamma}-rays using a pulsed 'white'-neutron source, coupled to a high-energy-resolution germanium-detector array. The excitation functions can unambiguously assign {gamma}-rays to a specific reaction product. Results from all these methods bridge the gaps in the systematics of high-spin states between the neutron-deficient and neutron-rich nuclei. Results near shell closures should motivate new shell model calculations.

  6. Magnetic excitations from an S=1/2 diamond-shaped tetramer compound Cu2PO4OH

    DOE PAGESBeta

    Matsuda, Masaaki; Dissanayake, Sachith E.; Abernathy, Douglas L.; Totsuka, K.; Belik, A. A.

    2015-11-30

    Inelastic neutron scattering experiments have been carried out on a powder sample of Cu2PO4OH, which consists of diamond-shaped tetramer spin units with S=1/2. We have observed two nearly dispersionless magnetic excitations at E1 ~2 and E2 ~0 meV, whose energy width are broader than the instrumental resolution. The simplest square tetramer model with one dominant interaction, which predicts two sharp excitation peaks at E1 and E2(=2E1), does not explain the experimental result. We found that two diagonal intratetramer interactions compete with the main interaction and weak intertetramer interactions connect the tetramers. The main intratetramer interaction is found to split intomore » two inequivalent ones due to a structural distortion below 160 K. Cu2PO4OH is considered to be a good material to study the S=1/2 Heisenberg tetramer system.« less

  7. A comparison between ``second-sphere effects'' in the excited state properties of coordination compounds and nonmolecular solids

    NASA Astrophysics Data System (ADS)

    Blasse, G.; Sabbatini, N.

    1987-09-01

    In this paper we compare second-sphere effects as known from the field of photochemistry and photophysics of coordination compounds with similar phenomena in nonmolecular solids. Literature data, as well as new results, especially on cryptates, are used. The similarity between these phenomena in both classes of compounds is much larger than thought at first glance and has been overlooked for the most part. The following effects are considered: the influence of complex encapsulation on the yield of photochemical processes and the thermal quenching temperature of luminescence; the interaction in ion pairs resulting in new energy levels and luminescence quenching; and the influence of electric charges on the position of absorption bands. Since quantitative calculations of these effects are not easy to perform, it is beneficial to discuss information available from different fields of research.

  8. Excitation of compound states in subsystems as an indirect tool in nuclear astrophysics. The theory of the Trojan Horse method

    SciTech Connect

    Mukhamedzhanov, A. M.

    2010-03-01

    Astrophysical reactions proceeding through compound states represent one of the crucial part of nuclear astrophysics. However, due to the presence of the Coulomb barrier, it is often very difficult or even impossible to obtain the astrophysical S(E) factor from measurements in the laboratory at astrophysically relevant energies. The Trojan Horse method (THM) provides a unique tool to obtain the information about resonant astrophysical reactions at astrophysical energies. Here the theory and application of the THM for the resonant reactions is addressed.

  9. Cosmogenic nuclei

    NASA Technical Reports Server (NTRS)

    Raisbeck, G. M.

    1986-01-01

    Cosmogenic nuclei, nuclides formed by nuclear interactions of galactic and solar cosmic rays with extraterrestrial or terrestrial matter are discussed. Long lived radioactive cosmogenic isotopes are focused upon. Their uses in dating, as tracers of the interactions of cosmic rays with matter, and in obtaining information on the variation of primary cosmic ray flux in the past are discussed.

  10. Properties of Products Originating from the Interaction of 35-MeV/nucleon {sup 7}Li Ions with Pb Nuclei

    SciTech Connect

    Demekhina, N.A.; Karapetyan, G.S.; Lukyanov, S.M.; Penionzhkevich, Yu.E.; Skobelev, N.K.; Yakushev, A.B.

    2005-01-01

    The results are presented that were obtained by measuring and analyzing the yields and kinematical features of radioactive products of the reactions initiated in a lead target by lithium ions accelerated to an energy of 35 MeV per nucleon. The cross sections, charge and mass distributions, and kinematical and energy features of various reaction products associated with the fission and the evaporation channels of the decay of excited nuclei are determined. Quantities that are calculated in the present study include the momenta and kinetic energies of residual nuclei, as well as the momentum transfer and the excitation energy of intermediate nuclear systems formed upon complete and incomplete fusion. On the basis of an analysis of data obtained in our experiment, the total cross section for nuclear interaction and partial widths with respect to various channels of the decay of intermediate compound nuclei are determined in the energy range being investigated.

  11. Extended Locus of Regular Nuclei

    SciTech Connect

    Amon, L.; Casten, R. F.

    2007-04-23

    A new family of IBM Hamiltonians, characterized by certain parameter values, was found about 15 years ago by Alhassid and Whelan to display almost regular dynamics, and yet these solutions to the IBM do not belong to any of the known dynamical symmetry limits (vibrational, rotational and {gamma} - unstable). Rather, they comprise an 'Arc of Regularity' cutting through the interior of the symmetry triangle from U(5) to SU(3) where suddenly there is a decrease in chaoticity and a significant increase in regularity. A few years ago, the first set of nuclei lying along this arc was discovered. The purpose of the present work is to search more broadly in the nuclear chart at all nuclei from Z = 40 - 100 for other examples of such 'regular' nuclei. Using a unique signature for such nuclei involving energy differences of certain excited states, we have identified an additional set of 12 nuclei lying near or along the arc. Some of these nuclei are known to have low-lying intruder states and therefore care must be taken, however, in judging their structure. The regularity exhibited by nuclei near the arc presumably reflects the validity or partial validity of some new, as yet unknown, quantum number describing these systems and giving the regularity found for them.

  12. Fusion probability in heavy nuclei

    NASA Astrophysics Data System (ADS)

    Banerjee, Tathagata; Nath, S.; Pal, Santanu

    2015-03-01

    Background: Fusion between two massive nuclei is a very complex process and is characterized by three stages: (a) capture inside the potential barrier, (b) formation of an equilibrated compound nucleus (CN), and (c) statistical decay of the CN leading to a cold evaporation residue (ER) or fission. The second stage is the least understood of the three and is the most crucial in predicting yield of superheavy elements (SHE) formed in complete fusion reactions. Purpose: A systematic study of average fusion probability, , is undertaken to obtain a better understanding of its dependence on various reaction parameters. The study may also help to clearly demarcate onset of non-CN fission (NCNF), which causes fusion probability, PCN, to deviate from unity. Method: ER excitation functions for 52 reactions leading to CN in the mass region 170-220, which are available in the literature, have been compared with statistical model (SM) calculations. Capture cross sections have been obtained from a coupled-channels code. In the SM, shell corrections in both the level density and the fission barrier have been included. for these reactions has been extracted by comparing experimental and theoretical ER excitation functions in the energy range ˜5 %-35% above the potential barrier, where known effects of nuclear structure are insignificant. Results: has been shown to vary with entrance channel mass asymmetry, η (or charge product, ZpZt ), as well as with fissility of the CN, χCN. No parameter has been found to be adequate as a single scaling variable to determine . Approximate boundaries have been obtained from where starts deviating from unity. Conclusions: This study quite clearly reveals the limits of applicability of the SM in interpreting experimental observables from fusion reactions involving two massive nuclei. Deviation of from unity marks the beginning of the domain of dynamical models of fusion. Availability of precise ER cross

  13. A compilation of information on the {sup 31}P(p,{alpha}){sup 28}Si reaction and properties of excited levels in the compound nucleus {sup 32}S

    SciTech Connect

    Miller, R.E.; Smith, D.L.

    1997-11-01

    This report documents a survey of the literature, and provides a compilation of data contained therein, for the {sup 31}P(p,{alpha}){sup 28}Si reaction. Attention is paid here to resonance states in the compound-nuclear system {sup 32}S formed by {sup 31}P + p, with emphasis on the alpha-particle decay channels, {sup 28}Si + {alpha} which populate specific levels in {sup 28}Si. The energy region near the proton separation energy for {sup 32}S is especially important in this context for applications in nuclear astrophysics. Properties of the excited states in {sup 28}Si are also considered. Summaries of all the located references are provided and numerical data contained in them are compiled in EXFOR format where applicable.

  14. Contributions of excited {sup 6}Li and {sup 7}Li nuclei to the production of {sup 4}He+{sup 2}H and {sup 4}He+{sup 3}H systems in {sup 16}O{sub p} collisions at a momentum of 3.25 GeV/c per nucleon

    SciTech Connect

    Olimov, K.; Glagolev, V. V.; Gulamov, K. G.; Lutpullaev, S. L.; Kurbanov, A. R.; Olimov, A. K.; Petrov, V. I.; Yuldashev, A. A.

    2013-07-15

    New experimental data on the cross sections for the yield of excited {sup 6}Li* and {sup 7}Li* nuclei and on their contributions to the production of {sup 4}He + {sup 2}H and {sup 4}He+{sup 3}H light dinuclear systems in {sup 16}O{sub p} collisions at a momentumof 3.25 A GeV/c per nucleon are presented.

  15. Spectroscopy of Neutron-rich Pu Nuclei

    SciTech Connect

    Chowdhury, P.; Hota, S.; Lakshmi, S.; Tandel, S. K.; Harrington, T.; Jackson, E.; Moran, K.; Shirwadkar, U.; Ahmad, I.; Carpenter, M. P.; Greene, J.; Hoffman, C. R.; Janssens, R. V. F.; Khoo, T. L.; Kondev, F. G.; Lauritsen, T.; Lister, C. J.; McCutchan, E. A.; Seweryniak, D.; Stefanescu, I.

    2011-10-28

    Spectroscopic studies of nuclei in the A{approx}250, Z{approx}100 region provide critical input to theoretical models that attempt to describe the structure and stability of the heaviest elements. We report here on new spectroscopic studies in the N = 150,151 nuclei {sup 244,245}Pu. (Z = 94). Excitations in these nuclei on the neutron-rich side of the valley of stability, accessed via inelastic and transfer reactions, complement fusion-evaporation studies of Z{>=}100 nuclei. States in {sup 244,245}Pu were populated using {sup 47}Ti and {sup 208}Pb beams incident on a {sup 244}Pu target, with delayed and prompt gamma rays detected by the Gammasphere array. The new results are discussed in the context of emerging systematics of one- and two-quasiparticle excitations in N{>=}150 nuclei.

  16. {gamma}-vibrational states in superheavy nuclei

    SciTech Connect

    Sun Yang; Long Guilu; Al-Khudair, Falih; Sheikh, Javid A.

    2008-04-15

    Recent experimental advances have made it possible to study excited structure in superheavy nuclei. The observed states have often been interpreted as quasiparticle excitations. We show that in superheavy nuclei collective vibrations systematically appear as low-energy excitation modes. By using the microscopic Triaxial Projected Shell Model, we make a detailed prediction on {gamma}-vibrational states and their E2 transition probabilities to the ground state band in fermium and nobelium isotopes where active structure research is going on, and in {sup 270}Ds, the heaviest isotope where decay data have been obtained for the ground-state and for an isomeric state.

  17. Quantum Monte Carlo calculations of light nuclei

    SciTech Connect

    Pieper, S.C.

    1998-12-01

    Quantum Monte Carlo calculations using realistic two- and three-nucleon interactions are presented for nuclei with up to eight nucleons. We have computed the ground and a few excited states of all such nuclei with Greens function Monte Carlo (GFMC) and all of the experimentally known excited states using variational Monte Carlo (VMC). The GFMC calculations show that for a given Hamiltonian, the VMC calculations of excitation spectra are reliable, but the VMC ground-state energies are significantly above the exact values. We find that the Hamiltonian we are using (which was developed based on {sup 3}H,{sup 4}He, and nuclear matter calculations) underpredicts the binding energy of p-shell nuclei. However our results for excitation spectra are very good and one can see both shell-model and collective spectra resulting from fundamental many-nucleon calculations. Possible improvements in the three-nucleon potential are also be discussed. {copyright} {ital 1998 American Institute of Physics.}

  18. Quantum Monte Carlo calculations of light nuclei

    SciTech Connect

    Pieper, Steven C.

    1998-12-21

    Quantum Monte Carlo calculations using realistic two- and three-nucleon interactions are presented for nuclei with up to eight nucleons. We have computed the ground and a few excited states of all such nuclei with Greens function Monte Carlo (GFMC) and all of the experimentally known excited states using variational Monte Carlo (VMC). The GFMC calculations show that for a given Hamiltonian, the VMC calculations of excitation spectra are reliable, but the VMC ground-state energies are significantly above the exact values. We find that the Hamiltonian we are using (which was developed based on {sup 3}H,{sup 4}He, and nuclear matter calculations) underpredicts the binding energy of p-shell nuclei. However our results for excitation spectra are very good and one can see both shell-model and collective spectra resulting from fundamental many-nucleon calculations. Possible improvements in the three-nucleon potential are also be discussed.

  19. Quantum Monte Carlo calculations of light nuclei.

    SciTech Connect

    Pieper, S. C.

    1998-08-25

    Quantum Monte Carlo calculations using realistic two- and three-nucleon interactions are presented for nuclei with up to eight nucleons. We have computed the ground and a few excited states of all such nuclei with Greens function Monte Carlo (GFMC) and all of the experimentally known excited states using variational Monte Carlo (VMC). The GFMC calculations show that for a given Hamiltonian, the VMC calculations of excitation spectra are reliable, but the VMC ground-state energies are significantly above the exact values. We find that the Hamiltonian we are using (which was developed based on {sup 3}H, {sup 4}He, and nuclear matter calculations) underpredicts the binding energy of p-shell nuclei. However our results for excitation spectra are very good and one can see both shell-model and collective spectra resulting from fundamental many-nucleon calculations. Possible improvements in the three-nucleon potential are also be discussed.

  20. Exotic Nuclei

    SciTech Connect

    Galindo-Uribarri, Alfredo {nmn}

    2010-01-01

    Current experimental developments on the study of exotic nuclei far from the valley of stability are discussed. I start with general aspects related to the production of radioactive beams followed by the description of some of the experimental tools and specialized techniques for studies in reaction spectroscopy, nuclear structure research and nuclear applications with examples from selected topical areas with which I have been involved. I discuss some of the common challenges faced in Accelerator Mass Spectrometry (AMS) and Radioactive Ion Beam (RIB) science.

  1. Properties of fission fragments for Z =112 -116 superheavy nuclei

    NASA Astrophysics Data System (ADS)

    Kaur, Gurjit; Sandhu, Kirandeep; Sharma, Manoj K.

    2016-07-01

    The dynamical cluster decay model (DCM) is applied to understand the dynamics of 48Ca+238U,244Pu,248Cm reactions at comparable excitation energies across the barrier. To understand the capture stage of *286112 ,*292114 , and *296116 nuclei, the compound nucleus formation probability is calculated. The indication of PC N<1 in the DCM framework demonstrates the fact that some competing process such as quasifission may occur at the capture stage of the 48Ca induced reactions. To understand this further, the comparative decay analysis of *286112 ,*292114 and *296116 , nuclei is carried out using β2 i deformations within hot optimum orientation criteria, and the calculated fission cross sections find nice agreement with available data. The fission mass distribution shows a double humped structure where a symmetric peak observed around the Sn region appears to find its genesis in a symmetric quasifission component. On the other hand, the emergence of peaks around Pb in the decay of Z =112 , 114, and 116 nuclei signify the possible presence of asymmetric quasifission. Higher and broader asymmetric quasifission peaks are observed for *296116 and *292114 nuclei as compared to *286112 nucleus. Beside this, the total kinetic energy (TKE) distribution of the decay fragments is also explored by using different proximity potentials, such as Prox-77, Prox-88, and Prox-00. Prox-88 seems to perform better and the calculated TKE values find relatively better comparison at lower angular momentum states. The possible role of different radii of the decaying nuclei is also exercised to understand the TKE ¯ dynamics of 48Ca+238U,244Pu,248Cm reactions.

  2. Electronic structure, transport properties, and excited states in CoTiSb, CoZrSb, and CoHfSb half-Heusler compounds

    NASA Astrophysics Data System (ADS)

    Janotti, Anderson; Gui, Zhigang; Kawasaki, Jason; Palmstrom, Chris; Himmetoglu, Burak

    CoTiSb is a member of a large family of half-Heusler compounds with 18 valence electrons. CoTiSb is semiconductor material with a band gap a little over 1 eV, and it has been considered promising for thermoelectric applications. It can be grown on conventional III-V semiconductors, and could potentially be integrated in III-V devices. Here we present results of first-principles calculations of electronic structure, transport properties, and excited states in CoTiSb, as well as CoZrSb and CoHfSb. Electronic structures are studied using density functional theory within the local density approximation, hybrid functional and quasiparticle GW methods. Both room-temperature Seebeck coefficient and carrier mobility are calculated from first-principles. We also determine the band alignments to III-V semiconductors, and all the results are presented and discussed in the light of available experimental data. This work was supported by the DOE.

  3. Theoretical study of the nuclear spin-molecular rotation coupling for relativistic electrons and non-relativistic nuclei. II. Quantitative results in HX (X = H,F,Cl,Br,I) compounds.

    PubMed

    Aucar, I Agustín; Gómez, Sergio S; Melo, Juan I; Giribet, Claudia C; Ruiz de Azúa, Martín C

    2013-04-01

    In the present work, numerical results of the nuclear spin-rotation (SR) tensor in the series of compounds HX (X = H,F,Cl,Br,I) within relativistic 4-component expressions obtained by Aucar et al. [J. Chem. Phys. 136, 204119 (2012)] are presented. The SR tensors of both the H and X nuclei are discussed. Calculations were carried out within the relativistic Linear Response formalism at the Random Phase Approximation with the DIRAC program. For the halogen nucleus X, correlation effects on the non-relativistic values are shown to be of similar magnitude and opposite sign to relativistic effects. For the light H nucleus, by means of the linear response within the elimination of the small component approach it is shown that the whole relativistic effect is given by the spin-orbit operator combined with the Fermi contact operator. Comparison of "best estimate" calculated values with experimental results yield differences smaller than 2%-3% in all cases. The validity of "Flygare's relation" linking the SR tensor and the NMR nuclear magnetic shielding tensor in the present series of compounds is analyzed. PMID:23574208

  4. Theoretical study of the nuclear spin-molecular rotation coupling for relativistic electrons and non-relativistic nuclei. II. Quantitative results in HX (X=H,F,Cl,Br,I) compounds

    NASA Astrophysics Data System (ADS)

    Aucar, I. Agustín; Gómez, Sergio S.; Melo, Juan I.; Giribet, Claudia C.; Ruiz de Azúa, Martín C.

    2013-04-01

    In the present work, numerical results of the nuclear spin-rotation (SR) tensor in the series of compounds HX (X=H,F,Cl,Br,I) within relativistic 4-component expressions obtained by Aucar et al. [J. Chem. Phys. 136, 204119 (2012), 10.1063/1.4721627] are presented. The SR tensors of both the H and X nuclei are discussed. Calculations were carried out within the relativistic Linear Response formalism at the Random Phase Approximation with the DIRAC program. For the halogen nucleus X, correlation effects on the non-relativistic values are shown to be of similar magnitude and opposite sign to relativistic effects. For the light H nucleus, by means of the linear response within the elimination of the small component approach it is shown that the whole relativistic effect is given by the spin-orbit operator combined with the Fermi contact operator. Comparison of "best estimate" calculated values with experimental results yield differences smaller than 2%-3% in all cases. The validity of "Flygare's relation" linking the SR tensor and the NMR nuclear magnetic shielding tensor in the present series of compounds is analyzed.

  5. The Peculiarities of the Production and Decay of Superheavy Nuclei

    SciTech Connect

    Itkis, M. G.; Bogachev, A. A.; Itkis, I. M.; Jandel, M.; Kliman, J.; Knyazheva, G. N.; Kondratiev, N. A.; Kozulin, E. M.; Krupa, L.; Oganessian, Yu. Ts.; Pokrovsky, I. V.; Prokhorova, E. V.; Rusanov, A. Ya.; Sagaidak, R. N.; Beghini, S.; Montagnoli, G.; Scarlassara, F.; Behera, B. R.; Corradi, L.; Fioretto, E.

    2006-08-14

    The interest in the study of the fission process of superheavy nuclei mainly deals with the opportunity to obtain information about the cross-section of the compound nucleus (CN) formation at excitation energies E*{approx_equal}15-30 MeV. It allows one to estimate the survival probability of the superheavy composite system after evaporation of 1-3 neutrons, i.e. in 'cold' or 'warm' fusion reactions. However, in order to solve this problem deeper understanding of the coalescence processes between colliding nuclei, the competition between fusion-fission and quasi-fission processes is needed. The characteristics of both processes, their manifestation in the experimental observables and the relative contribution to the capture cross-section in dependence on the excitation energies, reaction entrance channel etc were investigated for a wide range of target-projectile combinations. Results of the experiments devoted to the study of the fusion-fission and quasi-fission processes in the reactions of the formation of the superheavy nuclei with Z = 102-122 are presented. The heavy ions 26Mg, 48Ca, 50Ti, 58Fe and 64Ni were used as projectiles. The choice of the reactions with 48Ca and actinide-targets was inspired by the experiments on the production of the isotopes 283112, 289114 and 283116 in Dubna using the same reactions. The 50Ti, 58Fe and 64Ni projectiles were chosen since the corresponding projectile-target combinations lead to the synthesis of even heavier elements. The experiments were carried out at the U-400 accelerator of the Flerov Laboratory of Nuclear Reactions (JINR, Russia) and the XTU Tandem accelerator of the National Laboratory of Legnaro (LNL, Italy) using the time-of-flight spectrometer of fission fragments CORSET. The role of the shell effects, the influence of the entrance channel asymmetry and the deformations of colliding nuclei on the mechanism of the fusion-fission and the competitive process of quasi-fission are discussed. The recent results on

  6. Synthesis and Decay Properties of Superheavy Nuclei

    NASA Astrophysics Data System (ADS)

    Oganessian, Yu. Ts.; Utyonkov, V. K.; Lobanov, Yu. V.; Abdullin, F. Sh.; Polyakov, A. N.; Shirokovsky, I. V.; Tsyganov, Yu. S.; Gulbekian, G. G.; Bogomolov, S. L.; Gikal, B. N.; Mezentsev, A. N.; Iliev, S.; Subbotin, V. G.; Sukhov, A. M.; Voinov, A. A.; Buklanov, G. V.; Subotic, K.; Zagrebaev, V. I.; Itkis, M. G.; Patin, J. B.; Moody, K. J.; Wild, J. F.; Stoyer, M. A.; Stoyer, N. J.; Shaughnessy, D. A.; Kenneally, J. M.; Wilk, P. A.; Lougheed, R. W.

    2005-09-01

    We have studied the dependence of the production cross sections of the isotopes 282,283112 and 286-288114 on the excitation energy of the compound nuclei 286112 and 290114. The maximum cross sections of the xn-evaporation channels for the reaction 238U(48Ca,xn)286-x112 were measured to be: σ 3n = 2.5{ - 1.1}{ + 1.8} pb and σ 4n = 0.6{ - 0.5}{ + 1.6} pb ; for the reaction 242Pu(48Ca,xn)290-x114: σ2n 0.5 pb, σ 3n = 3.6{ - 1.7}{ + 3.4} pb and σ 4n = 4.5{ - 1.9}{ + 3.6} pb . In the reaction 233U(48Ca,2-4n)277-279112 we measured an upper cross section limit of σxn≤0.6 pb. An increase of σER in the reactions of actinide targets with 48Ca is consistent with the expected increase of the survivability of the excited compound nucleus upon closer approach to the closed neutron shell N=184. The observed nuclear decay properties of the nuclides with Z=104-118 are compared with theoretical nuclear mass calculations and the systematic trends of α-decay properties. As a whole, they give a consistent pattern of decay of the 18 even-Z neutron-rich nuclides with Z=104-118 and N=163-177.

  7. Collisions of deformed nuclei and superheavy-element production

    SciTech Connect

    Iwamoto, Akira; Moeller, P. |||; Nix, J.R.; Sagawa, Hiroyuki, Sagawa

    1995-09-01

    A detailed understanding of complete fusion cross sections in heavy-ion collisions requires a consideration of the effects of the deformation of the projectile and target. The aim here is to show that deformation and orientation of the colliding nuclei have a very significant effect on the fusion-barrier height and on the compactness of the touching configuration. To facilitate discussions of fusion configurations of deformed nuclei, the authors develop a classification scheme and introduce a notation convention for these configurations. They discuss particular deformations and orientations that lead to compact touching configurations and to fusion-barrier heights that correspond to fairly low excitation energies of the compound systems. Such configurations should be the most favorable for producing superheavy elements. They analyze a few projectile-target combinations whose deformations allow favorable entrance-channel configurations and whose proton and neutron numbers lead to compound systems in a part of the superheavy region where a half-lives are calculated to be observable, that is, longer than 1 {micro}s.

  8. Onset of quenching of the giant dipole resonance at high excitation energies

    NASA Astrophysics Data System (ADS)

    Santonocito, D.; Blumenfeld, Y.; Agodi, C.; Alba, R.; Bellia, G.; Coniglione, R.; Delaunay, F.; Del Zoppo, A.; Finocchiaro, P.; Hongmei, F.; Lima, V.; Maiolino, C.; Migneco, E.; Piattelli, P.; Sapienza, P.; Scarpaci, J. A.; Wieland, O.

    2014-11-01

    The evolution of the giant dipole resonance (GDR) properties in nuclei of mass A =120 to 132 has been investigated in an excitation energy range between 150 and 270 MeV through the study of complete and nearly complete fusion reactions using 116Sn beams at 17 A and 23 A MeV from the cyclotron of the Laboratorio Nazionale del Sud impinging on 12C and 24Mg targets. γ rays and light charged particles were detected using the multi-element detector array MEDEA in coincidence with evaporation residues detected by using mass and charge identification spectrometry with telescope (MACISTE). Light-charged-particle energy spectra were analyzed within the framework of a multiple-source-emission scenario by using a fitting procedure to determine the amount of pre-equilibrium emission and deduce the excitation energies reached in the compound nuclei. A detailed analysis of the γ -ray spectra and their comparison with statistical model calculations is presented. Evidence of a quenching of the GDR gamma yield was found at 270 MeV excitation energy. The quenching effect becomes progressively more important with increasing excitation energy, as observed when the comparison is extended to data from the reaction 36Ar+96Mo at 37 A MeV where hot nuclei were populated up to 430 MeV excitation energy. A coherent scenario emerges indicating the existence of a limiting excitation energy for the collective motion of about E*/A =2.1 MeV for systems of mass A =105 to 111 while a slightly lower value was observed for nuclei of mass A ˜132 . The existence of a possible link between GDR disappearance and the liquid-gas phase transition is discussed.

  9. Synthesis of superheavy elements and dinuclear-system concept of compound-nucleus formation

    SciTech Connect

    Antonenko, N.V.; Adamian, G.G.; Cherepanov, E.A.

    1996-12-31

    Dinuclear system concept is applied to the analysis of reactions used for the synthesis of elements with Z = 110, 112, 114, and 116. The inner fusion barriers obtained for these reactions are in good agreement with the experimental estimations resulted from the excitation energies of compound nuclei. A model is suggested for the calculation of the competition between complete fusion and quasifission in reactions with heavy nuclei. The fusion rate through the inner fusion barrier in mass asymmetry is found by using the multidimensional Kramers-type stationary solution of the Fokker-Planck equation. The influence of dissipative effects on the dynamics of nuclear fusion is considered.

  10. IBA in deformed nuclei

    SciTech Connect

    Casten, R.F.; Warner, D.D.

    1982-01-01

    The structure and characteristic properties and predictions of the IBA in deformed nuclei are reviewed, and compared with experiment, in particular for /sup 168/Er. Overall, excellent agreement, with a minimum of free parameters (in effect, two, neglecting scale factors on energy differences), was obtained. A particularly surprising, and unavoidable, prediction is that of strong ..beta.. ..-->.. ..gamma.. transitions, a feature characteristically absent in the geometrical model, but manifest empirically. Some discrepancies were also noted, principally for the K=4 excitation, and the detailed magnitudes of some specific B(E2) values. Considerable attention is paid to analyzing the structure of the IBA states and their relation to geometric models. The bandmixing formalism was studied to interpret both the aforementioned discrepancies and the origin of the ..beta.. ..-->.. ..gamma.. transitions. The IBA states, extremely complex in the usual SU(5) basis, are transformed to the SU(3) basis, as is the interaction Hamiltonian. The IBA wave functions appear with much simplified structure in this way as does the structure of the associated B(E2) values. The nature of the symmetry breaking of SU(3) for actual deformed nuclei is seen to be predominantly ..delta..K=0 mixing. A modified, and more consistent, formalism for the IBA-1 is introduced which is simpler, has fewer free parameters (in effect, one, neglecting scale factors on energy differences), is in at least as good agreement with experiment as the earlier formalism, contains a special case of the 0(6) limit which corresponds to that known empirically, and appears to have a close relationship to the IBA-2. The new formalism facilitates the construction of contour plots of various observables (e.g., energy or B(E2) ratios) as functions of N and chi/sub Q/ which allow the parameter-free discussion of qualitative trajectories or systematics.

  11. Understanding nuclei in the upper sd - shell

    SciTech Connect

    Sarkar, M. Saha; Bisoi, Abhijit; Ray, Sudatta; Kshetri, Ritesh; Sarkar, S.

    2014-08-14

    Nuclei in the upper-sd shell usually exhibit characteristics of spherical single particle excitations. In the recent years, employment of sophisticated techniques of gamma spectroscopy has led to observation of high spin states of several nuclei near A ≃ 40. In a few of them multiparticle, multihole rotational states coexist with states of single particle nature. We have studied a few nuclei in this mass region experimentally, using various campaigns of the Indian National Gamma Array setup. We have compared and combined our empirical observations with the large-scale shell model results to interpret the structure of these nuclei. Indication of population of states of large deformation has been found in our data. This gives us an opportunity to investigate the interplay of single particle and collective degrees of freedom in this mass region.

  12. True ternary fission of superheavy nuclei

    SciTech Connect

    Zagrebaev, V. I.; Karpov, A. V.; Greiner, Walter

    2010-04-15

    True ternary fission with formation of a heavy third fragment is quite possible for superheavy nuclei because of the strong shell effects leading to a three-body clusterization with the two doubly magic tinlike cores. The simplest way to discover this phenomenon in the decay of excited superheavy nuclei is a detection of two tinlike clusters with appropriate kinematics in low-energy collisions of medium-mass nuclei with actinide targets. The three-body quasi-fission process could be even more pronounced for giant nuclear systems formed in collisions of heavy actinide nuclei. In this case a three-body clusterization might be proved experimentally by the detection of two coincident leadlike fragments in low-energy U + U collisions.

  13. Star formation around active galactic nuclei

    NASA Technical Reports Server (NTRS)

    Keel, William C.

    1987-01-01

    Active galactic nuclei (Seyfert nuclei and their relatives) and intense star formation can both deliver substantial amounts of energy to the vicinity of a galactic nucleus. Many luminous nuclei have energetics dominated by one of these mechanisms, but detailed observations show that some have a mixture. Seeing both phenomena at once raises several interesting questions: (1) Is this a general property of some kinds of nuclei? How many AGNs have surround starbursts, and vice versa? (2) As in 1, how many undiscovered AGNs or starbursts are hidden by a more luminous instance of the other? (3) Does one cause the other, and by what means, or do both reflect common influences such as potential well shape or level of gas flow? (4) Can surrounding star formation tell us anything about the central active nuclei, such as lifetimes, kinetic energy output, or mechanical disturbance of the ISM? These are important points in the understanding of activity and star formation in galactic nuclei. Unfortunately, the observational ways of addressing them are as yet not well formulated. Some preliminary studies are reported, aimed at clarifying the issues involved in study of the relationships between stellar and nonstellar excitement in galactic nuclei.

  14. Superdeformation in the mercury nuclei

    SciTech Connect

    Janssens, R.V.F.; Carpenter, M.P.; Fernandez, P.B.; Moore, E.F.; Ahmad, I.; Khoo, T.L.; Wolfs, F.L.H. ); Drigert, M.W. ); Ye, D.; Beard, K.B.; Garg, U.; Reviol, W. ); Bearden, I.G.; Benet, P.; Daly, P.J.; Grabowski, Z.W. )

    1990-01-01

    We shall first summarize the present experimental situation concerning {sup 192}Hg, the nucleus regarded as the analog of {sup 152}Dy for this superdeformation (SD) region in that gaps are calculated to occur at large deformation for Z = 80 and N = 112. Proton and neutron excitations out of the {sup 192}Hg core will then be reviewed with particular emphasis on {sup 191}Hg and {sup 193}Tl. The presentation will conclude with a brief discussion on limits of the SD region for neutron deficient Hg nuclei. 26 refs., 10 figs.

  15. Exotic nuclei and nuclear forces

    NASA Astrophysics Data System (ADS)

    Otsuka, Takaharu

    2013-01-01

    evolution affects shapes of nuclei through Jahn-Teller-type mechanism, and a very interesting example with exotic Si isotopes is discussed. The third type of nuclear force is a three-body force, which originates in the Δ particle excitation as proposed by Fujita and Miyazawa many years ago. This force is shown to produce a repulsive interaction between valence neutrons after averaging effects from the third nucleon in the core. The same three-body force is responsible for neutron stars. By including such effects of the three-body force, one can predict the correct drip line of oxygen isotopes, for instance. Thus, the landscape of atomic nuclei varies in going from stable to exotic nuclei due to particular nuclear forces, leading to a paradigm shift. This paper overviews some basic ideas and selected examples.

  16. The Elusive Excited Quintet [superscript 5]D of Tb(III): A Source of Luminescence and Resonance Energy Transfer in Terbium Compounds

    ERIC Educational Resources Information Center

    Klier, Kamil

    2010-01-01

    The understanding of electronic structure of atomic and molecular term states involved in spectroscopic transitions is aided by projecting combinations of micro-configurations to multi-electron states with "good" quantum numbers of angular momenta. In rare-earth (RE) compounds, atomic term labels are justifiably carried over to compounds, because…

  17. NUCLEI AT HIGH ANGULAR MOMENTUM

    SciTech Connect

    Diamond, R.M.; Stephens, F.S.

    1980-06-01

    It appears that most nuclei show a compromise between purely collective and purely non-collective behavior at very high spins.non~collective behavior in nuclei has been seen only as high as 36 or 37{bar h}, at which point a more collective structure seems to develop. The concepts underlying the study of high angular momentum states are discussed. The factors that limit angular momentum in nuclei are considered. The currently emerging state of physics of very high spin states is reviewed. The detailed calculations currently made for high spin states are described, focusing not on the calculations themselves, but on the physical input to them and results that come out. Production of high-spin states using heavy-ion reactions is reviewed. Studies of {gamma}-rays de-exciting the evaporation residues from heavy-ion reactions are covered. Two types of {gamma} rays occur: those that cool the nucleus to or toward the yrast line, called "statistical," and those that are more or less parallel to the yrast line and remove the angular momentum, called "yrast~like." Collective rotation, in simplest form the motion of a deformed nucleus around an axis perpendicular to its symmetry axis, is also covered.

  18. Production of new superheavy Z=108-114 nuclei with {sup 238}U, {sup 244}Pu, and {sup 248,250}Cm targets

    SciTech Connect

    Feng Zhaoqing; Jin Genming; Li Junqing

    2009-11-15

    Within the framework of the dinuclear system (DNS) model, production cross sections of new superheavy nuclei with charged numbers Z=108-114 are analyzed systematically. Possible combinations based on the actinide nuclides {sup 238}U, {sup 244}Pu, and {sup 248,250}Cm with the optimal excitation energies and evaporation channels are pointed out to synthesize new isotopes that lie between the nuclides produced in the cold fusion reactions and the {sup 48}Ca-induced fusion reactions experimentally, which are feasible to be constructed experimentally. It is found that the production cross sections of superheavy nuclei decrease drastically with the charged numbers of compound nuclei. Larger mass asymmetries of the entrance channels enhance the cross sections in 2n-5n channels.

  19. Cryogenic exciter

    SciTech Connect

    Bray, James William; Garces, Luis Jose

    2012-03-13

    The disclosed technology is a cryogenic static exciter. The cryogenic static exciter is connected to a synchronous electric machine that has a field winding. The synchronous electric machine is cooled via a refrigerator or cryogen like liquid nitrogen. The static exciter is in communication with the field winding and is operating at ambient temperature. The static exciter receives cooling from a refrigerator or cryogen source, which may also service the synchronous machine, to selected areas of the static exciter and the cooling selectively reduces the operating temperature of the selected areas of the static exciter.

  20. Weak Interactions of Hot Nuclei in Stellar Collapse

    NASA Astrophysics Data System (ADS)

    Misch, Gordon Wendell

    The physics of the atomic nucleus and supernovas are fundamental to our very being. Indeed, supernovas provide the wind that disperses the nuclei of which we are composed, and the physics of nuclei is pivotal in supernova dynamics. During supernova core collapse, the extremely high temperatures and densities and low entropy favor large, neutron-rich nuclei at high excitation energy. My collaborators and I examine two weak interactions that occur in nuclei under these conditions. First, we study the production of neutrino pairs via de-excitation of hot nuclei. In de-exciting, the nucleus can emit a virtual Z0 boson that decays into a neutrino-antineutrino pair. We find this to be the dominant source of neutrino pairs of all flavors during collapse. Second, we use modern shell model computation techniques to revise the Brink-Axel hypothesis method of computing electron capture rates that was pioneered by Fuller, Fowler, and Newman. Our results show that the Brink-Axel hypothesis (which posits that the bulk of nuclear transition strength is distributed among transition energies independently of initial excitation energy) fails at low and moderate excitation, but that at high initial energies, the strength is largely independent of excitation. The failure of the Brink-Axel hypothesis manifests as the redistribution of strength to low and negative transition energies, which can have the effect of increasing the overall electron capture rate in the core.

  1. Excitations and possible bound states in the S = {1/2} alternating chain compound (VO){sub 2}P{sub 2}O{sub 7}

    SciTech Connect

    Tennant, D.A.; Nagler, S.E.; Sales, B.C.

    1997-07-30

    Magnetic excitations in an array of (VO){sub 2}P{sub 2}O{sub 7} single crystals have been measured using inelastic neutron scattering. Until now, (VO){sub 2}P{sub 2}O{sub 7} has been thought of as a two-leg antiferromagnetic Heisenberg spin ladder with chains running in the a-direction. The present results show unequivocally that (VO){sub 2}P{sub 2}O{sub 7} is best described as an alternating spin-chain directed along the crystallographic b-direction. In addition to the expected magnon with magnetic zone-center energy gap {Delta} = 3.1 meV, a second excitation is observed at an energy just below 2{Delta}. The higher mode may be a triplet two-magnon bound state. Numerical results in support of bound modes are presented.

  2. Properties of Haldane Excitations and Multiparticle States in the Antiferromagnetic Spin-1 Chain Compound CsNiCl3

    SciTech Connect

    Kenzelmann, M.; Cowley, R. A.; Buyers, W. J. L.; Tun, Z.; Coldea, Radu; Enderle, M.

    2002-01-01

    We report inelastic time-of-flight and triple-axis neutron scattering measurements of the excitation spectrum of the coupled antiferromagnetic spin-1 Heisenberg chain system CsNiCl{sub 3}. Measurements over a wide range of wave-vector transfers along the chain confirm that above T{sub N} CsNiCl{sub 3} is in a quantum-disordered phase with an energy gap in the excitation spectrum. The spin correlations fall off exponentially with increasing distance with a correlation length {zeta} = 4.0(2) sites at T = 6.2K. This is shorter than the correlation length for an antiferromagnetic spin-1 Heisenberg chain at this temperature, suggesting that the correlations perpendicular to the chain direction and associated with the interchain coupling lower the single-chain correlation length. A multiparticle continuum is observed in the quantum-disordered phase in the region in reciprocal space where antiferromagnetic fluctuations are strongest, extending in energy up to twice the maximum of the dispersion of the well-defined triplet excitations. We show that the continuum satisfies the Hohenberg-Brinkman sum rule. The dependence of the multiparticle continuum on the chain wave vector resembles that of the two-spinon continuum in antiferromagnetic spin-1/2 Heisenberg chains. This suggests the presence of spin-1/2 degrees of freedom in CsNiCl{sub 3} for T {approx}< 12 K, possibly caused by multiply frustrated interchain interactions.

  3. Extended similarity transformed equation-of-motion coupled cluster theory (extended-STEOM-CC): Applications to doubly excited states and transition metal compounds

    NASA Astrophysics Data System (ADS)

    Nooijen, Marcel; Lotrich, Victor

    2000-07-01

    The diagonalization manifold in similarity transformed equation-of-motion coupled cluster (STEOM-CC) theory is extended to include doubly excited determinants. In the resulting extended-STEOM approach accurate results are obtained for doubly excited states in small model systems for which full configuration interaction (CI) benchmark results are available (˜0.1 eV errors). On the other hand, extended-STEOM results are found to be virtually identical (<0.1 eV shifts) to the original STEOM results for states that are dominated by single excitations, at least in prototypical organic molecules. The extended-STEOM method is also applied to the transition metal complexes TiCl4, Ni(CO)4, and MnO4-, and yields improved results compared to STEOM and EOM-CCSD. For highly correlated systems, like the permangenate anion, results are not yet fully satisfactory however. In these cases the dominant source of error appears to be the description of ground, ionized, and attached states that underly the similarity transformed Hamiltonian in the extended-STEOM approach.

  4. Mathematical simulation of the amplification of 1790-nm laser radiation in a nuclear-excited He – Ar plasma containing nanoclusters of uranium compounds

    SciTech Connect

    Kosarev, V A; Kuznetsova, E E

    2014-02-28

    The possibility of applying dusty active media in nuclearpumped lasers has been considered. The amplification of 1790-nm radiation in a nuclear-excited dusty He – Ar plasma is studied by mathematical simulation. The influence of nanoclusters on the component composition of the medium and the kinetics of the processes occurring in it is analysed using a specially developed kinetic model, including 72 components and more than 400 reactions. An analysis of the results indicates that amplification can in principle be implemented in an active laser He – Ar medium containing 10-nm nanoclusters of metallic uranium and uranium dioxide. (lasers)

  5. Alpha-cluster model of atomic nuclei

    NASA Astrophysics Data System (ADS)

    Sosin, Zbigniew; Błocki, Jan; Kallunkathariyil, Jinesh; Łukasik, Jerzy; Pawłowski, Piotr

    2016-05-01

    The description of a nuclear system in its ground state and at low excitations based on the equation of state (EoS) around normal density is presented. In the expansion of the EoS around the saturation point, additional spin polarization terms are taken into account. These terms, together with the standard symmetry term, are responsible for the appearance of the α-like clusters in the ground-state configurations of the N = Z even-even nuclei. At the nuclear surface these clusters can be identified as alpha particles. A correction for the surface effects is introduced for atomic nuclei. Taking into account an additional interaction between clusters the binding energies and sizes of the considered nuclei are very accurately described. The limits of the EoS parameters are established from the properties of the α, 3He and t particles.

  6. Is Fusion Inhibited for Weakly Bound Nuclei?

    SciTech Connect

    Takahashi, J.; Munhoz, M.; Szanto, E.M.; Carlin, N.; Added, N.; Suaide, A.A.; de Moura, M.M.; Liguori Neto, R.; Szanto de Toledo, A.; Canto, L.F.

    1997-01-01

    Complete fusion of light radioactive nuclei is predicted to be hindered at near-barrier energies. This feature is investigated in the case of the least bound stable nuclei. Evaporation residues resulting from the {sup 6,7}Li+{sup 9}Be and {sup 6,7}Li+{sup 12}C fusion reactions have been measured in order to study common features in reactions involving light weakly bound nuclei. The experimental excitation functions revealed that the fusion cross section is significantly smaller than the total reaction cross section and also smaller than the fusion cross section expected from the available systematics. A clear correlation between the fusion probability and nucleon (cluster) separation energy has been established.The results suggest that the breakup process has a strong influence on the hindrance of the fusion cross section. {copyright} {ital 1996} {ital The American Physical Society}

  7. Application of recent double-hybrid density functionals to low-lying singlet-singlet excitation energies of large organic compounds

    NASA Astrophysics Data System (ADS)

    Meo, F. Di; Trouillas, P.; Adamo, C.; Sancho-García, J. C.

    2013-10-01

    The present work assesses some recently developed double-hybrid density functionals (B2π-PLYP, PBE0-DH, and PBE0-2) using linear-response Tamm-Dancoff Time-Dependent Density Functional Theory. This assessment is achieved against experimentally derived low-lying excitation energies of large organic dyes of recent interest, including some excitations dominated by charge-transfer transitions. Comparisons are made with some of the best-performing methods established from the literature, such as PBE0 or B3LYP hybrid or the recently proposed B2-PLYP and B2GP-PLYP double-hybrid models, to ascertain their quality and robustness on equal footing. The accuracy of parameter-free or empirical forms of double-hybrid functionals is also briefly discussed. Generally speaking, it turns out that double-hybrid expressions always provide more accurate estimates than corresponding hybrid methods. Double-hybrid functionals actually reach averaged accuracies of 0.2 eV, that can be admittedly considered close to any intended accuracy limit within the present theoretical framework.

  8. Magnetic excitations from an S=1/2 diamond-shaped tetramer compound Cu2PO4OH

    SciTech Connect

    Matsuda, Masaaki; Dissanayake, Sachith E.; Abernathy, Douglas L.; Totsuka, K.; Belik, A. A.

    2015-11-30

    Inelastic neutron scattering experiments have been carried out on a powder sample of Cu2PO4OH, which consists of diamond-shaped tetramer spin units with S=1/2. We have observed two nearly dispersionless magnetic excitations at E1 ~2 and E2 ~0 meV, whose energy width are broader than the instrumental resolution. The simplest square tetramer model with one dominant interaction, which predicts two sharp excitation peaks at E1 and E2(=2E1), does not explain the experimental result. We found that two diagonal intratetramer interactions compete with the main interaction and weak intertetramer interactions connect the tetramers. The main intratetramer interaction is found to split into two inequivalent ones due to a structural distortion below 160 K. Cu2PO4OH is considered to be a good material to study the S=1/2 Heisenberg tetramer system.

  9. Changes in the structure of nuclei between the magic neutron numbers 50 and 82 as indicated by a rotating-cluster analysis of the energy values of the first 2j excited states of isotopes of cadmium

    SciTech Connect

    Pauling, L.

    1981-09-01

    Values of R, the radius of rotation of the rotating cluster, are calculated from the observed values of the energy of the lowest 2/sup +/ states of the even isotopes of Cd, Sn, and Te with the assumption that the cluster is ..cap alpha.., pb, and ..cap alpha.., respectively. R shows a maximum at approx. N = 58, a minimum at approx. N = 62, and a second maximum at approx. N = 70. The increase to the first maximum is interpreted as resulting from the overcrowding of spherons (alphas and tritons) in the mantle (outer layer) of the nuclei, causing the cluster to change from rotating in the mantle to skimming over its surface; the decrease to the minimum results from the addition of three dineutrons to the core, expanding the mantle and permitting the rotating cluster to begin to drop back into it; and the increase to the second maximum results from the overcrowding of the larger mantle surrounding the core containing the semimagic number 14 of neutrons rather than the magic numbers 8 for N = 50. The decrease after the second maximum results from the further increase in the number of core neutrons to 20, corresponding to the magic number 82. Some additional evidence for the change to an intermediate structure between N = 50 and N = 82 is also discussed.

  10. Mechanism of heavy ion fusion to superheavy nuclei

    NASA Astrophysics Data System (ADS)

    Adamian, Gurgen G.; Antonenko, Nikolai V.; Scheid, Werner

    2011-10-01

    This article reviews different models for the description of fusion of heavy ions to superheavy nuclei by using adiabatic and diabatic potentials. The dynamics of fusion is basically different in the two types of models for fusion: In the adiabatic models the nuclei melt together, whereas in the diabatic models the nuclei transfer nucleons between each other up to the instant when the compound nucleus is formed. As final result we state that diabatic potentials seem more appropriate for the description of fusion of heavy nuclei than adiabatic potentials.

  11. Fragmentation of spherical radioactive heavy nuclei as a novel probe of transient effects in fission

    SciTech Connect

    Schmitt, C.; Schmidt, K.-H.; Kelic, A.; Heinz, A.; Jurado, B.

    2010-06-15

    Peripheral collisions with radioactive heavy-ion beams at relativistic energies are discussed as an innovative approach for probing the transient regime experienced by fissile systems evolving toward quasiequilibrium and thereby studying the viscous nature of nuclear matter. A dedicated experiment using the advanced technical installations of GSI, Darmstadt, made it possible to realize ideal conditions for the investigation of relaxation effects in a metastable well. Combined with a highly sensitive experimental signature, it provides a measure of the transient effects with respect to the flux over the fission barrier. Within a two-step reaction process, 45 proton-rich unstable spherical isotopes between At and Th produced by projectile-fragmentation of a stable {sup 238}U beam have been used as secondary projectiles which impinge on lead target nuclei. The fragmentation of the radioactive projectiles results in nearly spherical compound nuclei that span a wide range in excitation energy and fissility. The decay of these excited systems by fission is studied with a dedicated setup which, together with the inverse kinematics of the reaction, permits the detection of both fission products in coincidence and the determination of their atomic numbers with high resolution. The information on the nuclear charges of the two fragments is used to sort the data according to the initial excitation energy and fissility of the compound nucleus. The width of the fission-fragment nuclear charge distribution is shown to be specifically sensitive to presaddle transient effects and is used to establish a clock for the passage of the saddle point. The comparison of the experimental results with model calculations points to a fission delay tau{sub trans} of (3.3+-0.7)x10{sup -21} s for initially spherical compound nuclei, independent of excitation energy and fissility. This value suggests a nuclear dissipation strength beta at small deformation of (4.5+-0.5)x10{sup 21} s{sup -1}. The

  12. Quantum Monte Carlo calculations for light nuclei.

    SciTech Connect

    Wiringa, R. B.

    1998-10-23

    Quantum Monte Carlo calculations of ground and low-lying excited states for nuclei with A {le} 8 are made using a realistic Hamiltonian that fits NN scattering data. Results for more than 40 different (J{pi}, T) states, plus isobaric analogs, are obtained and the known excitation spectra are reproduced reasonably well. Various density and momentum distributions and electromagnetic form factors and moments have also been computed. These are the first microscopic calculations that directly produce nuclear shell structure from realistic NN interactions.

  13. Invariant mass spectroscopy of halo nuclei

    SciTech Connect

    Nakamura, Takashi

    2008-11-11

    We have applied the invariant mass spectroscopy to explore the low-lying exited states of halo nuclei at intermediate energies around 70 MeV/nucleon at RIKEN. As examples, we show here the results of Coulomb breakup study for {sup 11}Li using the Pb target, as well as breakup reactions of {sup 14}Be with p and C targets. The former study revealed a strong Coulomb breakup cross section reflecting the large enhancement of E1 strength at low excitation energies (soft E1 excitation). The latter revealed the observation of the first 2{sup +} state in {sup 14}Be.

  14. Active galactic nuclei

    PubMed Central

    Fabian, Andrew C.

    1999-01-01

    Active galactic nuclei are the most powerful, long-lived objects in the Universe. Recent data confirm the theoretical idea that the power source is accretion into a massive black hole. The common occurrence of obscuration and outflows probably means that the contribution of active galactic nuclei to the power density of the Universe has been generally underestimated. PMID:10220363

  15. The formation and decay of superheavy nuclei produced in 48Ca-induced reactions

    NASA Astrophysics Data System (ADS)

    Kumar, Sushil; Balasubramaniam, M.; Gupta, Raj K.; Münzenberg, G.; Scheid, W.

    2003-04-01

    The formation of superheavy nuclei in 48Ca+232Th, 238U, 242,244Pu and 248Cm reactions and their subsequent decay are studied within the quantum mechanical fragmentation theory (QMFT) and the QMFT-based preformed cluster decay model (PCM) of Gupta and collaborators. According to QMFT, all these 48Ca-induced reactions are cold fusion reactions with relative excitation energies larger than those for the Pb-induced cold fusion reactions and smaller than those for the lighter beam, i.e. Mg, Si or S-induced hot fusion reactions. The same reactions were first suggested by Gupta et al in 1977 on the basis of QMFT, and this study re-establishes the same result. In fact, for such heavy isotopes of Z = 110 to 116, 50Ca is shown to be a better beam for cold fusion, but 50Ca is a radioactive nucleus. The alpha-decay half-lives of these nuclei after 3n and/or 4n evaporations, i.e. of the evaporation residues of these compound systems, calculated on PCM compare reasonably well with the experiments published by the Dubna group and another recent calculation. As expected for such rare decays, PCM calculations show that the alpha-preformation factors are small, ~10-8 to 10-10. The possible competition of alpha-decays with heavy cluster emissions from these superheavy nuclei is also probed from the point of view of searching for new nuclear structure information and possible future experiments with such exotic nuclei. The decay half-lives for some clusters are in fact shown to be lower than the limits of experiments for nuclei with enough available atoms.

  16. Soft radiative strength in warm nuclei

    SciTech Connect

    Becker, J A; Bernstein, L A; Garrett, P E; Nelson, R O; Schiller, A; Voinov, A; Agvaanluvsan, U; Algin, E; Belgya, T; Chankova, R; Guttormsen, M; Mitchell, G E; Rekstad, J; Siem, S

    2004-03-08

    Unresolved transitions in the nuclear {gamma}-ray cascade produced in the decay of excited nuclei are best described by statistical concepts: a continuous radiative strength function (RSF) and level density yield mean values of transition matrix elements. Data on the soft (E{sub {gamma}} < 3-4 MeV) RSF for transitions between warm states (i.e. states several MeV above the yrast line) have, however, remained elusive.

  17. Measurement of fusion excitation functions in the system {sup 78}Kr + {sup 100}Mo

    SciTech Connect

    Rehm, K.E.; Jiang, C.L.; Esbensen, H.

    1995-08-01

    Earlier measurements of fusion reactions involving {sup 78}Kr and {sup 100}Mo projectiles and Ni-targets showed surprisingly large fusion yields at low energies which could not be explained by coupled-channels calculations. The main difference to similar measurements involving the neighboring {sup 86}Kr and {sup 92}Mo isotopes was the different slope of the excitation functions at sub-barrier energies. An analysis of a variety of experiments showed a correlation between the nuclear structure and the slope of the excitation functions, with the {open_quotes}soft{close_quotes} transitional nuclei ({sup 78}Kr, {sup 100}Mo) exhibiting shallower slopes than the {open_quotes}stiff{close_quotes} nuclei ({sup 86}Kr, {sup 92}Mo) measured at the same energies with respect to the barrier. In this experiment we studied the fusion excitation function involving two transitional nuclei {sup 78}Kr + {sup 100}Mo. The measurements were performed with {sup 78}Kr beams from the ECR source at energies between 285-370 MeV. Separation of the evaporation nucleus from the elastically scattered particles was achieved by measuring time-of-flight and magnetic rigidity in the gas-filled spectrograph. The data were completely analyzed. A comparison of the cross sections with measurements for the system {sup 86}Kr + {sup 92}Mo populating the same compound nucleus {sup 178}Pt. It shows good agreement at the highest energies, but quite different falloffs of the excitation functions toward lower energies. Coupled-channels calculations, including multi-phonon excitation for the two systems, are being performed.

  18. Modeling level structures of odd-odd deformed nuclei

    SciTech Connect

    Hoff, R.W.; Kern, J.; Piepenbring, R.; Boisson, J.P.

    1985-01-15

    A technique for modeling quasiparticle excitation energies and rotational parameters in odd-odd deformed nuclei has been applied to actinide species where new experimental data have been obtained by use of neutron-capture gamma-ray spectroscopy. The input parameters required for the calculation were derived from empirical data on single-particle excitations in neighboring odd-mass nuclei. Calculated configuration-specific values for the Gallagher-Moszkowski splittings were used. Calculated and experimental level structures for /sup 238/Np, /sup 244/Am, and /sup 250/Bk are compared, as well as those for several nuclei in the rare-earch region. The agreement for the actinide species is excellent, with bandhead energies deviating 22 keV and rotational parameters 5%, on the average. Corresponding average deviations for five rare-earth nuclei are 47 keV and 7%. Several applications of this modeling technique are discussed.

  19. Modeling level structures of odd-odd deformed nuclei

    SciTech Connect

    Hoff, R.W.; Kern, J.; Piepenbring, R.; Boisson, J.P.

    1984-09-07

    A technique for modeling quasiparticle excitation energies and rotational parameters in odd-odd deformed nuclei has been applied to actinide species where new experimental data have been obtained by use of neutron-capture gamma-ray spectroscopy. The input parameters required for the calculation were derived from empirical data on single-particle excitations in neighboring odd-mass nuclei. Calculated configuration-specific values for the Gallagher-Moszkowski splittings were used. Calculated and experimental level structures for /sup 238/Np, /sup 244/Am, and /sup 250/Bk are compared, as well as those for several nuclei in the rare-earth region. The agreement for the actinide species is excellent, with bandhead energies deviating 22 keV and rotational parameters 5%, on the average. Corresponding average deviations for five rare-earth nuclei are 47 keV and 7%. Several applications of this modeling technique are discussed. 18 refs., 5 figs., 4 tabs.

  20. Light element production by low energy nuclei from massive stars

    NASA Technical Reports Server (NTRS)

    Vangioni-Flam, E.; Casse, M.; Ramaty, R.

    1997-01-01

    The Orion complex is a source of gamma rays attributed to the de-excitation of fast carbon and oxygen nuclei excited through interactions with ambient hydrogen and helium. This has consequences for the production and evolution of light isotopes in the Galaxy, as massive stars appear as prolific sources of C-O rich low energy nuclei. The different stages of massive star evolution are considered in relation to the acceleration of nuclei to moderate energies. It is concluded that the low energy nuclear component originating from massive stars plays a larger role than the usual Galactic cosmic rays in shaping the evolution of Li-6, Be-9, B-10 and B-11, especially in the early Galactic evolution. The enhancement of the B-11/B-10 ratio observed in meteorites and in the interstellar medium is attributed to the interaction of low energy carbon nuclei with ambient H and to a lesser degree, to neutrino spallation.

  1. Static and Statistical Properties of Hot Rotating Nuclei in a Macroscopic Temperature-Dependent Finite-Range Model

    SciTech Connect

    Ryabov, E.G.; Adeev, G.D.

    2005-09-01

    A macroscopic temperature-dependent model that takes into account nuclear forces of finite range is used to calculate the static and statistical properties of hot rotating compound nuclei. The level-density parameter is approximated by an expression of the leptodermous type. The resulting expansion coefficients are in good agreement with their counterparts proposed previously by A.V. Ignatyuk and his colleagues. The effect of taking simultaneously into account the temperature of a nucleus and its angular momentum on the quantities under study, such as the heights and positions of fission barriers and the effective moments of inertia of nuclei at the barrier, is considered, and the importance of doing this is demonstrated. The fissility parameter (Z{sup 2}/A){sub crit} and the position of the Businaro-Gallone point are studied versus temperature. It is found that, with increasing temperature, both parameters are shifted to the region of lighter nuclei. It is shown that the inclusion of temperature leads to qualitatively the same effects as the inclusion of the angular momentum of a nucleus, but, quantitatively, thermal excitation leads to smaller effects than rotational excitation.

  2. Alternating-parity collective states of yrast and nonyrast bands in lanthanide and actinide nuclei

    SciTech Connect

    Nadirbekov, M. S. Yuldasheva, G. A.; Denisov, V. Yu.

    2015-03-15

    Excited collective states of even-even nuclei featuring quadrupole and octupole deformations are studied within a nonadiabatic collective model with a Gaussian potential energy. Rotational states of the yrast band and vibrational-rotational states of nonyrast bands are considered in detail. The energies of alternating-parity excited states of the yrast band in the {sup 164}Er, {sup 220}Ra, and {sup 224}Th nuclei; the yrast and first nonyrast bands in the {sup 154}Sm and {sup 160}Gd nuclei; and the yrast, first nonyrast, and second nonyrast bands in the {sup 224}Ra and {sup 240}Pu nuclei are described well on the basis of the proposed model.

  3. Single particle versus collectivity, shapes of exotic nuclei

    NASA Astrophysics Data System (ADS)

    Jungclaus, Andrea

    2016-03-01

    In this article some selected topics of nuclear structure research will be discussed as illustration of the progress reached in this field during the last thirty years. These examples evidence the improvement of our understanding of the atomic nucleus reached on the basis of countless experiments, performed to study both exotic nuclei (nuclei far-off the valley of stability) as well as nuclei under exotic conditions (high excitation energy/temperature or large angular momentum/rotational frequency), using stable and radioactive ion beams. The experimental progress, in parallel to the advancement of modern theoretical descriptions, led us to a much richer view of this fundamental many-body system.

  4. Level densities and shell corrections of superheavy nuclei

    NASA Astrophysics Data System (ADS)

    Bezbakh, A. N.; Shneidman, T. M.; Adamian, G. G.; Antonenko, N. V.

    2015-02-01

    The intrinsic level densities of superheavy nuclei in the α-decay chains of 296;298;300120 nuclei are calculated using the single-particle spectra obtained with the modifed two-center shell model. The level density parameters are extracted and compared with their phenomenological values used in the calculations of the survival of excited heavy nuclei. The dependences of the level density parameters on the mass and charge numbers as well as on the ground-state shell corrections are studied.

  5. Fission of actinide nuclei using multi-nucleon transfer reactions

    NASA Astrophysics Data System (ADS)

    Léguillon, Romain; Nishio, Katsuhisa; Hirose, Kentaro; Orlandi, Riccardo; Makii, Hiroyuki; Nishinaka, Ichiro; Ishii, Tetsuro; Tsukada, Kazuaki; Asai, Masato; Chiba, Satoshi; Ohtsuki, Tsutomu; Araki, Shohei; Watanabe, Yukinobu; Tatsuzawa, Ryotaro; Takaki, Naoyuki

    2014-09-01

    We are promoting a campaign to measure fission-fragment mass distributions for neutron-rich actinide nuclei populated by transfer reactions from their ground state up to an excitation energy of several tens MeV. We thus obtain the excitation energy dependence of the mass distribution. The experiment was carried out at the 20 MV JAEA tandem facility at Tokai. We report on the data obtained in the direct reaction 18 O + 232 Th . Transfer-channels and excitation energies of the fissioning nuclei were identified using silicon dE-E detectors located at forward angle. Two fission fragments were detected in coincidence using multi-wire proportional counters. Fission fragment masses were determined by kinematic consideration. We obtained the fission fragment mass distributions for 13 nuclei from actinium to uranium and some fission barrier heights. We are promoting a campaign to measure fission-fragment mass distributions for neutron-rich actinide nuclei populated by transfer reactions from their ground state up to an excitation energy of several tens MeV. We thus obtain the excitation energy dependence of the mass distribution. The experiment was carried out at the 20 MV JAEA tandem facility at Tokai. We report on the data obtained in the direct reaction 18 O + 232 Th . Transfer-channels and excitation energies of the fissioning nuclei were identified using silicon dE-E detectors located at forward angle. Two fission fragments were detected in coincidence using multi-wire proportional counters. Fission fragment masses were determined by kinematic consideration. We obtained the fission fragment mass distributions for 13 nuclei from actinium to uranium and some fission barrier heights. Present study is supported by the Ministry of Education, Culture, Sports, Science and Technology of Japan.

  6. Clustering effects in 48Cr composite nuclei produced via the 24Mg+24Mg reaction

    NASA Astrophysics Data System (ADS)

    Di Nitto, A.; Vardaci, E.; Brondi, A.; La Rana, G.; Cinausero, M.; Gelli, N.; Moro, R.; Nadtochy, P. N.; Prete, G.; Vanzanella, A.

    2016-04-01

    The nuclear properties of 48Cr composite α -like nuclei produced at 60 MeV of excitation energy via the 24Mg+24Mg reaction were investigated. This excitation energy corresponds to a resonance with a narrow width (170 keV) observed in the elastic and inelastic channels, which was interpreted as a highly deformed state. To gain insight on the deformation of this state exclusive measurements of light charged particles were carried out with 8 π LP apparatus at Laboratori Nazionali di Legnaro and compared to statistical model predictions. The measured of α -particle energy spectra, α -evaporation residues, α -α , and α -α -α correlations indicate the limitation of the rotating liquid drop model in describing the nuclear shape of the compound nucleus along the decay cascade. To reproduce the full set of experimental data very elongated nuclear shapes had to be considered, with an axis ratio 3 :1 at the resonance angular momentum. This large deformation is consistent with previous findings for α -like nuclei and with the predictions of the cranked cluster model.

  7. Exotic Light Nuclei

    ERIC Educational Resources Information Center

    Cerny, Joseph; Poskanzer, Arthur M.

    1978-01-01

    Among the light elements, nuclei with unequal numbers of protons and neutrons are highly unstable. Some survive just long enough to be detected and exhibit unusual regimes of radioactive decay. ( Autor/MA)

  8. Few-Body Models of Light Nuclei

    NASA Astrophysics Data System (ADS)

    Ershov, S. N.; Vaagen, J. S.; Zhukov, M. V.

    2015-06-01

    Experiments confirm a variety of cluster structures in many light nuclei. The observation of nuclear halos at drip-lines has accentuated the question of the degrees of freedom for bound and low-lying continuum states. In these cases the many-body dynamics of nuclear structure may be well approximated by few-body cluster models that often suggest conceptually simple approaches explaining successfully many features of light nuclei. Thus few-body cluster models have been successfully used for description of the nuclear structure of weakly bound halo nuclei and their emergent cluster degrees of freedom. They have attractive features supplying in a most transparent way the asymptotic behavior and continuum properties of weakly bound systems. Such models assume a separation in internal cluster (core) degrees of freedom and the relative motion of few-body constituents. Such separation is only an approximation, and low-lying states appear where the core cannot be considered as inert system and additional degrees of freedom connected to excited core states have to be taken into account. For fixed total angular momentum a coupling to excited core states having different spins involves additional partial waves into the consideration. This allows to account for some emergent (collective) core degrees of freedom and gives a more realistic description of nuclear properties. It is an analogue to increasing the number of shells within the framework of shell-model approaches. Some examples from recent nuclear structure exploration within few-body halo cluster models are presented.

  9. The Onset of Deformation in Neutron-Deficient At Nuclei

    SciTech Connect

    Smith, M.B.; Chapman, R.; Cocks, J.F.C.; Dorvaux, O.; Helariutta, K.; Jones, P.M.; Julin, R.; Juutinen, S.; Kankaanpaa, H.; Kettunen, H.; Kuusiniemi, P.; Le Coz, Y.; Leino, M.; Middleton, D.J.; Muikku, M.; Nieminen, P.; Rahkila, P.; Savelius, A.; Spohr, K.-M.

    1999-12-31

    Excited states in the {sup 197}At nucleus have been identified for the first time using the recoil-decay-tagging technique. The excitation energy of these states is found to be consistent with the systematics of neutron-deficient At nuclei and with calculations indicating that the nucleus may be deformed in its ground state. A more recent experiment, to study states in {sup 195}At, is discussed.

  10. The onset of deformation in neutron-deficient At nuclei

    SciTech Connect

    Smith, M. B.; Chapman, R.; Middleton, D. J.; Spohr, K.-M.; Cocks, J. F. C.; Dorvaux, O.; Helariutta, K.; Jones, P. M.; Julin, R.; Juutinen, S.; Kankaanpaeae, H.; Kettunen, H.; Kuusiniemi, P.; Leino, M.; Muikku, M.; Nieminen, P.; Rahkila, P.; Savelius, A.; Coz, Y. Le

    1999-11-16

    Excited states in the {sup 197}At nucleus have been identified for the first time using the recoil-decay-tagging technique. The excitation energy of these states is found to be consistent with the systematics of neutron-deficient. At nuclei and with calculations indicating that the nucleus may be deformed in its ground state. A more recent experiment, to study states in {sup 195}At, is discussed.

  11. Self-consistent theory of finite Fermi systems vs Skyrme-Hartree-Fock method. Spherical nuclei

    NASA Astrophysics Data System (ADS)

    Saperstein, E. E.; Tolokonnikov, S. V.

    2016-01-01

    Recent results of the Fayans energy density functional (EDF) for spherical nuclei are reviewed. A comparison is made with predictions of several Skyrme EDFs. The charge radii and characteristics of the first 2+ excitations in semi-magic nuclei are briefly discussed. The single-particle spectra of doubly magic nuclei are considered in more detail. The phonon-particle coupling effects are analyzed including the tadpole term.

  12. Transition from collective to noncollective rotation at high spin in N approx. = 87 nuclei

    SciTech Connect

    Baktash, C.

    1982-01-01

    The systematics of the (E2) ..gamma.. ray transition energies and the available lifetime data are used to characterize the excitation modes of the light rare-earth nuclei (N greater than or equal to 82) at different spins. The results, which include our recently obtained data on /sup 149/Gd, /sup 154/Ho, /sup 155/Er, /sup 157/Yb and /sup 158/Yb nuclei, indicate that, at low spins, the nuclear excitation mode (shapes) change from single-particle excitations (weakly oblate) in N less than or equal to 85 nuclei to quasi-vibrational (soft triaxial) in N = 86, weakly rotational (prolate) in N = 87, and rotational (prolate) in the N greater than or equal to 88 systems. At higher angular momenta, all these nuclei show a general tendency to traverse the (epsilon,..gamma..) plane towards the oblate axis, and to eventually adopt the aligned coupling mode of excitation.

  13. Scattering Of Light Nuclei

    SciTech Connect

    Quaglioni, S; Navratil, P; Roth, R

    2009-12-15

    The exact treatment of nuclei starting from the constituent nucleons and the fundamental interactions among them has been a long-standing goal in nuclear physics. Above all nuclear scattering and reactions, which require the solution of the many-body quantum-mechanical problem in the continuum, represent an extraordinary theoretical as well as computational challenge for ab initio approaches.We present a new ab initio many-body approach which derives from the combination of the ab initio no-core shell model with the resonating-group method [4]. By complementing a microscopic cluster technique with the use of realistic interactions, and a microscopic and consistent description of the nucleon clusters, this approach is capable of describing simultaneously both bound and scattering states in light nuclei. We will discuss applications to neutron and proton scattering on sand light p-shell nuclei using realistic nucleon-nucleon potentials, and outline the progress toward the treatment of more complex reactions.

  14. The Subtleties of Pairing and Collective Structures in Deformed Nuclei

    NASA Astrophysics Data System (ADS)

    Sharpey-Schafer, J. F.

    2015-11-01

    It is well known that simple monopole pairing is a pretty crude approximation. It can account for the observations that the ground states of all even-even nuclei have spin-parity 01+ and that there is a pairing gap above the ground state in deformed nuclei before particle-hole configurations can be excited. As an approximation it is best for proton and neutron mid-shell nuclei where the available single particle Nilsson wavefunctions have large overlaps. However at the beginning of regions of deformation, where high-K orbitals can be bought to the Fermi surface from a lower shell, simple monopole pairing is inadequate in describing the physics of the observed data. More recently, with a considerable increase in the quantity and quality of experimental data available, configuration dependent pairing has been used to account for the properties of low-lying first excited 02+ states in N = 88 and 90 nuclei at the onset of deformation in the rare earths. The properties of 02+ states in these and other nuclei at the start of regions of deformation and the effects of blocking of pairing leading to a decrease in the backbending critical frequencies in odd nuclei are presented.

  15. Super-heavy nuclei

    NASA Astrophysics Data System (ADS)

    Hofmann, Sigurd

    2015-11-01

    Scientifically based searches for elements beyond uranium started after the discovery of the neutron. Neutrons captured by uranium nuclei and subsequent {β }- decay, similarly as most of the elements were produced in nature, was the successful method applied. However, as a first result, Hahn and Strassmann discovered nuclear fission indicating a limit for the existence of nuclei at an increasing number of protons. Eventually, the nuclear shell model allowed for a more accurate calculation of binding energies, half-lives and decay modes of the heaviest nuclei. Theoreticians predicted a region of increased stability at proton number Z = 126, later shifted to 114, and neutron number N = 184. These nuclei receive their stability from closed shells for the protons and neutrons. Later, increased stability was also predicted for deformed nuclei at Z = 108 and N = 162. In this review I will report on experimental work performed on research to produce and identify these super-heavy nuclei (SHN). Intensive heavy ion beams, sophisticated target technology, efficient electromagnetic ion separators, and sensitive detector arrays were the prerequisites for discovery of 12 new elements during the last 40 years. The results are described and compared with theoretical predictions and interpretations. An outlook is given on further improvement of experimental facilities which will be needed for exploration of the extension and structure of the island of SHN, in particular for searching for isotopes with longer half-lives predicted to be located in the south east of the island, for new elements, and last not least, for surprises which, naturally, emerge unexpectedly.

  16. On quadrupole vibrations in nearly spherical nuclei

    NASA Astrophysics Data System (ADS)

    Yates, S. W.

    2012-09-01

    A new understanding of low-lying quadrupole vibrations in nuclei is emerging through lifetime measurements performed with fast neutrons at the accelerator laboratory of the University of Kentucky in combination with high-sensitivity measurements with other probes. In the stable cadmium nuclei, which have long been considered to be the best examples of vibrational behavior, we find that many E2 transition probabilities are well below harmonic vibrator expectations, and the B(E2)s cannot be explained with calculations incorporating configuration mixing between vibrational phonon states and intruder excitations. These data place severe limits on the collective models, and it is suggested that the low-lying levels of the Cd isotopes may not be of vibrational origin. An additional example of an apparent quadrupole vibrational nucleus, 62Ni, is considered.

  17. Hadrons in Nuclei

    SciTech Connect

    Mosel, Ulrich

    2004-08-30

    Changes of hadronic properties in dense nuclear matter as predicted by theory have usually been investigated by means of relativistic heavy-ion reactions. In this talk I show that observable consequences of such changes can also be seen in more elementary reactions on nuclei. Particular emphasis is put on a discussion of photonuclear reactions; examples are the dilepton production at {approx_equal} 1 GeV and the hadron production in nuclei at 10-20 GeV photon energies. The observable effects are expected to be as large as in relativistic heavy-ion collisions and can be more directly related to the underlying hadronic changes.

  18. Superdeformed oblate superheavy nuclei

    SciTech Connect

    Jachimowicz, P.; Kowal, M.; Skalski, J.

    2011-05-15

    We study stability of superdeformed oblate (SDO) superheavy Z{>=}120 nuclei predicted by systematic microscopic-macroscopic calculations in 12D deformation space and confirmed by the Hartree-Fock calculations with the SLy6 force. We include into consideration high-K isomers that very likely form at the SDO shape. Although half-lives T{sub 1/2} < or approx. 10{sup -5} s are calculated or estimated for even-even spin-zero systems, decay hindrances known for high-K isomers suggest that some SDO superheavy nuclei may be detectable by the present experimental technique.

  19. Light nuclei production in fusion of heavy ions

    SciTech Connect

    Antonenko, N.V.; Ivanova, S.P.; Jolos, R.V.; Scheid, W. Joint Institute for Nuclear Research, 141980 Dubna )

    1994-10-01

    A possible mechanism of the production of light nuclei in fusion reactions is considered. It is shown that the decay of the dinuclear system during its evolution to a compound nucleus yields a substantial rate for the production of light nuclei. The cross section of this process is calculated for the reaction [sup 58]Ni+[sup 58]Ni. The coupling of other modes of motion causes an increase of the asymmetric decay of the dinuclear system.

  20. Photonuclear reactions of actinide and pre-actinide nuclei at intermediate energies

    SciTech Connect

    Mukhopadhyay, Tapan; Basu, D. N.

    2007-12-15

    Photonuclear reaction is described with an approach based on the quasideuteron nuclear photoabsorption model followed by the process of competition between light particle evaporation and fission for the excited nucleus. Thus fission process is considered as a decay mode. The evaporation-fission process of the compound nucleus is simulated in a Monte Carlo framework. Photofission reaction cross sections are analysed in a systematic manner in the energy range {approx}50-70 MeV for the actinides {sup 232}Th, {sup 233}U, {sup 235}U, {sup 238}U, and {sup 237}Np and the pre-actinide nuclei {sup 208}Pb and {sup 209}Bi. The study reproduces satisfactorily well the available experimental data of photofission cross sections at energies {approx}50-70 MeV and the increasing trend of nuclear fissility with the fissility parameter Z{sup 2}/A for the actinides and pre-actinides at intermediate energies ({approx}20-140 MeV)

  1. New approach to calculating the potential energy of colliding nuclei

    SciTech Connect

    Kurmanov, R. S.; Kosenko, G. I.

    2014-12-15

    The differential method proposed by the present authors earlier for the reduction of volume integrals in calculating the potential energy of a compound nucleus is generalized to the case of two interacting nuclei. The Coulomb interaction energy is obtained for the cases of a sharp and a diffuse boundary of nuclei, while the nuclear interaction energy is found only for nuclei with a sharp boundary, the finiteness of the nuclear-force range being taken into account. The present method of calculations permits reducing the time it takes to compute the potential energy at least by two orders of magnitude.

  2. Open s d -shell nuclei from first principles

    NASA Astrophysics Data System (ADS)

    Jansen, G. R.; Schuster, M. D.; Signoracci, A.; Hagen, G.; Navrátil, P.

    2016-07-01

    We extend the ab initio coupled-cluster effective interaction (CCEI) method to open-shell nuclei with protons and neutrons in the valence space and compute binding energies and excited states of isotopes of neon and magnesium. We employ a nucleon-nucleon and three-nucleon interaction from chiral effective field theory evolved to a lower cutoff via a similarity renormalization group transformation. We find good agreement with experiment for binding energies and spectra, while charge radii of neon isotopes are underestimated. For the deformed nuclei 20Ne and 24Mg, we reproduce rotational bands and electric quadrupole transitions within uncertainties estimated from an effective field theory for deformed nuclei, thereby demonstrating that collective phenomena in s d -shell nuclei emerge from complex ab initio calculations.

  3. Open sd-shell nuclei from first principles

    DOE PAGESBeta

    Jansen, Gustav R.; Signoracci, Angelo J.; Hagen, Gaute; Navratil, Petr

    2016-07-05

    We extend the ab initio coupled-cluster e ective interaction (CCEI) method to open-shell nuclei with protons and neutrons in the valence space, and compute binding energies and excited states of isotopes of neon and magnesium. We employ a nucleon-nucleon and three-nucleon interaction from chiral e ective eld theory evolved to a lower cuto via a similarity renormalization group transformation. We nd good agreement with experiment for binding energies and spectra, while charge radii of neon isotopes are underestimated. For the deformed nuclei 20Ne and 24Mg we reproduce rotational bands and electric quadrupole transitions within uncertainties estimated from an e ectivemore » eld theory for deformed nuclei, thereby demonstrating that collective phenomena in sd-shell nuclei emerge from complex ab initio calculations.« less

  4. Scissors mode of Gd nuclei studied from resonance neutron capture

    SciTech Connect

    Kroll, J.; Baramsai, B.; Becker, J. A.; and others

    2012-10-20

    Spectra of {gamma} rays following the neutron capture at isolated resonances of stable Gd nuclei were measured. The objectives were to get new information on photon strength of {sup 153,155-159}Gd with emphasis on the role of the M1 scissors-mode vibration. An analysis of the data obtained clearly indicates that the scissors mode is coupled not only to the ground state, but also to all excited levels of the nuclei studied. The specificity of our approach ensures unbiasedness in estimating the sumed scissors-mode strength {Sigma}B(M1){up_arrow}, even for odd product nuclei, for which conventional nuclear resonance fluorescence measurements yield only limited information. Our analysis indicates that for these nuclei the sum {Sigma}B(M1){up_arrow} increases with A and for {sup 157,159}Gd it is significantly higher compared to {sup 156,158}Gd.

  5. Applications of Skyrme energy-density functional to fusion reactions for synthesis of superheavy nuclei

    SciTech Connect

    Wang Ning; Scheid, Werner; Wu Xizhen; Liu Min; Li Zhuxia

    2006-10-15

    The Skyrme energy-density functional approach has been extended to study massive heavy-ion fusion reactions. Based on the potential barrier obtained and the parametrized barrier distribution the fusion (capture) excitation functions of a lot of heavy-ion fusion reactions are studied systematically. The average deviations of fusion cross sections at energies near and above the barriers from experimental data are less than 0.05 for 92% of 76 fusion reactions with Z{sub 1}Z{sub 2}<1200. For the massive fusion reactions, for example, the {sup 238}U-induced reactions and {sup 48}Ca+{sup 208}Pb, the capture excitation functions have been reproduced remarkably well. The influence of structure effects in the reaction partners on the capture cross sections is studied with our parametrized barrier distribution. By comparing the reactions induced by double-magic nucleus {sup 48}Ca and by {sup 32}S and {sup 35}Cl, the ''threshold-like'' behavior in the capture excitation function for {sup 48}Ca-induced reactions is explored and an optimal balance between the capture cross section and the excitation energy of the compound nucleus is studied. Finally, the fusion reactions with {sup 36}S, {sup 37}Cl, {sup 48}Ca, and {sup 50}Ti bombarding {sup 248}Cm, {sup 247,249}Bk, {sup 250,252,254}Cf, and {sup 252,254}Es, as well as the reactions leading to the same compound nucleus with Z=120 and N=182, are studied further. The calculation results for these reactions are useful for searching for the optimal fusion configuration and suitable incident energy in the synthesis of superheavy nuclei.

  6. Octupole collectivity in nuclei

    NASA Astrophysics Data System (ADS)

    Butler, P. A.

    2016-07-01

    The experimental and theoretical evidence for octupole collectivity in nuclei is reviewed. Recent theoretical advances, covering a wide spectrum from mean-field theory to algebraic and cluster approaches, are discussed. The status of experimental data on the behaviour of energy levels and electric dipole and electric octupole transition moments is reviewed. Finally, an outlook is given on future prospects for this field.

  7. Quark structure of nuclei

    SciTech Connect

    Blankenbecler, R.

    1981-01-01

    A brief review is given of selected topics involved in the relativistic quark structure of nuclei such as the infinite momentum variables, scaling variables, counting rules, forward-backward variables, thermodynamic-like limit, QCD effects, higher quark bags, confinement, and many unanswered questions.

  8. Physics with Polarized Nuclei.

    ERIC Educational Resources Information Center

    Thompson, William J.; Clegg, Thomas B.

    1979-01-01

    Discusses recent advances in polarization techniques, specifically those dealing with polarization of atomic nuclei, and how polarized beams and targets are produced. These techniques have greatly increased the scope of possible studies, and provided the tools for testing fundamental symmetries and the spin dependence of nuclear forces. (GA)

  9. The Structure of Nuclei Far from Stability

    SciTech Connect

    Zganjar, E.F.

    1999-02-25

    From among a number of important nuclear structure results that have emerged from our research program during the past few years, two stand out as being of extra significance. These are: (a) the identification of a diabatic coexisting structure in {sup 187}Au which arises solely from differences in proton occupation of adjacent oscillator shells, and (b) the realization of a method for estimating EO strength in nuclei and the resulting prediction that the de-excitation of superdeformed bands may proceed, in some cases, by strong EO transitions.

  10. Excited Delirium

    PubMed Central

    Takeuchi, Asia; Ahern, Terence L.; Henderson, Sean O.

    2011-01-01

    Excited (or agitated) delirium is characterized by agitation, aggression, acute distress and sudden death, often in the pre-hospital care setting. It is typically associated with the use of drugs that alter dopamine processing, hyperthermia, and, most notably, sometimes with death of the affected person in the custody of law enforcement. Subjects typically die from cardiopulmonary arrest, although the cause is debated. Unfortunately an adequate treatment plan has yet to be established, in part due to the fact that most patients die before hospital arrival. While there is still much to be discovered about the pathophysiology and treatment, it is hoped that this extensive review will provide both police and medical personnel with the information necessary to recognize and respond appropriately to excited delirium. PMID:21691475

  11. Energetic Nuclei, Superdensity and Biomedicine

    ERIC Educational Resources Information Center

    Baldin, A. M.

    1977-01-01

    High-energy, relativistic nuclei were first observed in cosmic rays. Studing these nuclei has provided an opportunity for analyzing the composition of cosmic rays and for experimentally verifying principles governing the behavior of nuclear matter at high and super-high temperatures. Medical research using accelerated nuclei is suggested.…

  12. Excited baryons

    SciTech Connect

    Mukhopadhyay, N.C.

    1986-01-01

    The status of the theory of the low-energy approach to hadron structure is reviewed briefly by surveying a few relevant models. A few examples of tests needed to sort out the predictions of different models pertaining to the quark-gluon structure of hadrons are discussed, and given the resulting physics objectives, a few experimental options for excited baryon research at CFBAF are suggested. (LEW)

  13. Decay analysis of pre-actinide and trans-actinide nuclei formed using various projectiles on a 197Au target at ECN*=60 MeV

    NASA Astrophysics Data System (ADS)

    Grover, Neha; Kaur, Gurvinder; Sharma, Manoj K.

    2016-01-01

    The collective clusterization approach of the dynamical cluster decay model (DCM) has been applied to study the decay of odd mass nuclei 223Pa*, 215Fr*, 227Np*, and 233Am*, which are formed in heavy-ion-induced reactions. The aim of this study is to investigate the decay pattern and related behavior of these heavy mass nuclei formed in four distinct reactions involving different projectiles (with mass A =18 -36 ) induced on 197Au target nucleus. Further, in order to analyze the role of deformations, the calculations have been done by considering spherical choice of fragmentation as well as with inclusion of quadrupole (β2) deformation. For the heavy mass region, with fission being the dominant decay mode, an attempt has been made to investigate the effect of projectile mass in reference to fission decay patterns of the pre-actinide 215Fr* nucleus and the trans-actinide nuclei 227Np* 223Pa*, 223Am* and formed at common excitation energy, ECN*=60 MeV . Besides this, the shell closure effects and the role of orientation have been explored, which suggest the presence of a noncompound nucleus process such as quasifission (QF) for the odd mass nuclei under consideration. For both the compound nucleus and the noncompound nucleus processes, the results obtained using DCM are found to have nice agreement with experimental observations. The isotopic and isobaric analysis is also worked out so as to have a comprehensive idea about the dynamics involved.

  14. Comment on breakup densities of hot nuclei

    NASA Astrophysics Data System (ADS)

    Viola, V. E.; Kwiatkowski, K.; Yennello, S. J.; Natowitz, J. B.

    2006-06-01

    In [V.E. Viola et al., Phys. Rev. Lett. 93 (2004) 132701, D.S. Bracken et al., Phys. Rev. C 69 (2004) 034612] the observed decrease in spectral peak energies of IMFs emitted from hot nuclei was interpreted in terms of a breakup density that decreased with increasing excitation energy. Subsequently, Raduta et al. [Ad. Raduta et al., Phys. Lett. B 623 (2005) 43] performed MMM simulations that showed decreasing spectral peaks could be obtained at constant density. In this Letter we point out that this apparent inconsistency is due to a selective comparison of theory and data that overlooks the evolution of the fragment multiplicities as a function of excitation energy.

  15. The scission point configuration of fissioning nuclei

    NASA Astrophysics Data System (ADS)

    Ivanyuk, Fedir

    2016-06-01

    We define the optimal shape which fissioning nuclei attain just before the scission and calculate the deformation energy as function of the mass asymmetry at the scission point. The calculated deformation energy is used in quasi-static approximation for the estimation of mass distribution, total kinetic and excitation energy of fission fragments, and the total number of prompt neutrons. The calculated results reproduce rather well the experimental data on the position of the peaks in the mass distribution of fission fragments, the total kinetic and excitation energy of fission fragments. The calculated value of neutron multiplicity is somewhat larger than experimental results. The saw-tooth structure of neutron multiplicity is qualitatively reproduced.

  16. Selective estrogen receptor-beta (SERM-beta) compounds modulate raphe nuclei tryptophan hydroxylase-1 (TPH-1) mRNA expression and cause antidepressant-like effects in the forced swim test.

    PubMed

    Clark, J A; Alves, S; Gundlah, C; Rocha, B; Birzin, E T; Cai, S-J; Flick, R; Hayes, E; Ho, K; Warrier, S; Pai, L; Yudkovitz, J; Fleischer, R; Colwell, L; Li, S; Wilkinson, H; Schaeffer, J; Wilkening, R; Mattingly, E; Hammond, M; Rohrer, S P

    2012-11-01

    Estrogen acts through two molecularly distinct receptors termed estrogen receptor alpha (ERα) and estrogen receptor beta (ERβ) which bind estradiol with similar affinities and mediate the effects of estrogen throughout the body. ERα plays a major role in reproductive physiology and behavior, and mediates classic estrogen signaling in such tissues as the uterus, mammary gland, and skeleton. ERβ, however, modulates estrogen signaling in the ovary, the immune system, prostate, gastrointestinal tract, and hypothalamus, and there is some evidence that ERβ can regulate ERα activity. Moreover, ERβ knockout studies and receptor distribution analyses in the CNS suggest that this receptor may play a role in the modulation of mood and cognition. In recent years several ERβ-specific compounds (selective estrogen receptor beta modulators; SERM-beta) have become available, and research suggests potential utility of these compounds in menopausal symptom relief, breast cancer prevention, diseases that have an inflammatory component, osteoporosis, cardiovascular disease, and inflammatory bowel disease, as well as modulation of mood, and anxiety. Here we demonstrate an antidepressant-like effect obtained using two SERM-beta compounds, SERM-beta1 and SERM-beta2. These compounds exhibit full agonist activity at ERβ in a cell based estrogen response element (ERE) transactivation assay. SERM-beta1 and 2 are non-proliferative with respect to breast as determined using the MCF-7 breast cancer cell-based assay and non-proliferative in the uterus as determined by assessing the effects of SERM-beta compounds on immature rat uterine weight and murine uterine weight. In vivo SERM-beta1 and 2 are brain penetrant and display dose dependent efficacy in the murine dorsal raphe assays for induction of tryptophan hydroxylase mRNA and progesterone receptor protein. These compounds show activity in the murine forced swim test and promote hippocampal neurogenesis acutely in rats. Taken

  17. Transverse momenta of fragments of relativistic sulfur and lead nuclei after their interaction with track-emulsion nuclei at energies of 200 and 160 GeV per nucleon

    SciTech Connect

    Lepekhin, F. G. Tkach, L. N.

    2011-05-15

    Transverse-momentum distributions of doubly charged fragments of sulfur and lead nuclei having energies of 200 and 160 GeV per nucleon and interacting with nuclei in a track emulsion were investigated. No trace of compression or heating of nuclear matter in the interaction of these nuclei with track-emulsion nuclei was revealed experimentally. Transverse momenta of fragments of relativistic nuclei were found to obey a normal distribution that corresponds to a degenerate momentum distribution of nucleons in the ground state of a nucleus before its interaction with a track-emulsion nucleus. There is no piece of evidence that fragments of relativistic nuclei originate from some excited state of an intermediate nucleus. This picture of the fragmentation of relativistic nuclei complies with the naive parton model proposed by Feynman and Gribov. In summary, the fragmentation of relativistic nuclei at energies of 160 and 200 GeV per nucleon is cold and fast.

  18. Nuclear excitations at constant temperature

    SciTech Connect

    Voinov, A. V.; Oginni, B. M.; Grimes, S. M.; Brune, C. R.; Massey, T. N.; Schiller, A.; Guttormsen, M.; Larsen, A. C.; Siem, S.

    2009-03-15

    Neutron and proton evaporation spectra from the {sup 6}Li+{sup 55}Mn and d+{sup 59}Co reactions have been analyzed with the Hauser-Feshbach approach using different input models for nuclear level densities of {sup 60}Ni and {sup 60}Co nuclei. It has been found that models with a Fermi-gas like temperature dependence fail to reproduce particle spectra from both reactions simultaneously. We obtained the surprising result that the only way to describe our data is to assume the independence of the nuclear temperature on the excitation energy up to about the 20 MeV energy range.

  19. Space Shuttle ice nuclei

    NASA Technical Reports Server (NTRS)

    Turco, R. P.; Toon, O. B.; Whitten, R. C.; Cicerone, R. J.

    1982-01-01

    Estimates are made showing that, as a consequence of rocket activity in the earth's upper atmosphere in the Shuttle era, average ice nuclei concentrations in the upper atmosphere could increase by a factor of two, and that an aluminum dust layer weighing up to 1000 tons might eventually form in the lower atmosphere. The concentrations of Space Shuttle ice nuclei (SSIN) in the upper troposphere and lower stratosphere were estimated by taking into account the composition of the particles, the extent of surface poisoning, and the size of the particles. Calculated stratospheric size distributions at 20 km with Space Shuttle particulate injection, calculated SSIN concentrations at 10 and 20 km altitude corresponding to different water vapor/ice supersaturations, and predicted SSIN concentrations in the lower stratosphere and upper troposphere are shown.

  20. Nuclei in Astrophysics

    NASA Astrophysics Data System (ADS)

    Penionzhkevich, Yu. E.

    2016-06-01

    This work is an attempt to present some problems on the evolution of the Universe: the nucleosynthesis and cosmochronology from the standpoint of physics of particles and nuclei, in particular with the use of the latest results, obtained by means of radioactive nuclear beams. The comparison is made between the processes taking place in the Universe and the mechanisms of formation and decay of nuclei, as well as of their interaction at different energies. Examples are given to show the capabilities of nuclearphysics methods for studying cosmic objects and properties of the Universe. The results of investigations in nuclear reactions, induced by radioactive nuclear beams, make it possible to analyze the nucleosynthesis scenario in the region of light elements in a new manner.

  1. Exotic phenomena in nuclei

    NASA Astrophysics Data System (ADS)

    Neff, Thomas; Feldmeier, Hans; Roth, Robert

    2006-10-01

    In the Fermionic Molecular Dynamics (FMD) model the nuclear many-body system is described using Slater determinants with Gaussian wave-packets as single-particle states. The flexibility of the FMD wave functions allows for a consistent description of shell model like structures, deformed states, cluster structures as well as halos. An effective interaction derived from the realistic Argonne V18 interaction using the Unitary Correlation Operator Method is used for all nuclei. Results for nuclei in the p-shell will be presented. Halo features are present in the Helium isotopes, cluster structures are studied in Beryllium and Carbon isotopes. The interplay between shell structure and cluster structures in the ground and the Hoyle state in ^12C will be discussed.

  2. Isotopic dependence of the cross section for the induced fission of heavy nuclei

    SciTech Connect

    Bolgova, O. N.; Adamian, G. G.; Antonenko, N. V.; Zubov, A. S.; Ivanova, S. P.; Scheid, W.

    2009-06-15

    The cross sections for the induced fission of {sup 211-223}Ra, {sup 203-211}Rn, and {sup 221-231}Th nuclei undergoing peripheral collisions with {sup 208}Pb nuclei are calculated on the basis of the statistical model. The role of the N = 126 neutron shell is studied. The level density in excited nuclei is determined within the Fermi gas model and a model that takes into account the collective enhancement of the level density. The inclusion of a particle-hole excitation in addition to a collective Coulomb excitation makes it possible to obtain a satisfactory description of experimental cross sections for the fission of radium isotopes. The calculated ratios of the cross sections for the induced fission of {sup 236}U ({sup 237}U) and {sup 238}U ({sup 239}U) nuclei agree with experimental data.

  3. Pairing forces in nuclei

    SciTech Connect

    Chasman, R.R.

    1996-12-31

    In this contribution, the author mentions some features of pairing forces that are unique to nuclei and cover some areas of major interest in nuclear structure research, that involve pairing. At the level of most nuclear structure studies, nuclei are treated as consisting of two kinds of fermions (protons and neutrons) in a valence space with rather few levels. These features give rise to unique aspects of pairing forces in nuclei: (1) n-p pairing in T = 0 as well as the usual T = 1 pairing that is characteristic of like fermions; (2) a need to correct pairing calculations for the (1/N) effects that can typically be neglected in superconducting solids. An issue of current concern is the nature of the pairing interaction: several recent studies suggest a need for a density dependent form of the pairing interaction. There is a good deal of feedback between the questions of accurate calculations of pairing interactions and the form and magnitude of the pairing interaction. Finally, the authors discuss some many-body wave functions that are a generalization of the BCS wave function form, and apply them to a calculation of energy level spacings in superdeformed rotational bands.

  4. Pygmy Dipole Strength and Neutron Skins in Exotic Nuclei

    NASA Astrophysics Data System (ADS)

    Klimkiewicz, A.; Paar, N.; Adrich, P.; Fallot, M.; Boretzky, K.; Aumann, T.; Cortina-Gil, D.; Pramanik, U. Datta; Elze, Th. W.; Emling, H.; Geissel, H.; Hellström, M.; Jones, K. L.; Kratz, J. V.; Kulessa, R.; Nociforo, C.; Palit, R.; Simon, H.; Surówka, G.; Sümmerer, K.; Vretenar, D.; Waluś, W.

    2008-05-01

    Dipole strength distributions were determined for the neutron-rich nuclei 129-132Sn and 133,134Sb from electromagnetic excitation in an experiment using the FRS-LAND setup. For all nuclei, a sizeable fraction of ``pygmy'' dipole strength at excitation energies well below the giant dipole resonance was observed. The integrated low-lying dipole strength of the nuclei with low neutron separation energies can be compared to results for stable nuclei (e.g. N = 82 isotopes) determined for the energy regime of 5-9 MeV. A clear increase of the dipole strength with increasing asymmetry of the nuclei is observed. Comparing the ratio of the low-lying dipole over the giant dipole strength to recent relativistic mean field calculations, values for the parameters a4 and p0 of the symmetry energy and for the neutron skin thickness are derived. Averaged over 130Sn and 132Sn we extract a4 = 31.8+/-1.3 MeV and p0 = 2.2+/-0.5 MeV/fm3. The neutron skin sizes are determined to Rn-Rp = 0.23+/-0.03 fm and 0.24+/-0.03 fm for 130Sn and 132Sn, respectively. For 208Pb a neutron skin thickness of Rn-Rp = 0.18+/-0.035 fm follows, when applying the same method and using earlier published experimental findings on the dipole strength.

  5. Sexual excitement.

    PubMed

    Stoller, R J

    1976-08-01

    Sexual excitement depends on a scenario the person to be aroused has been writing since childhood. The story is an adventure, an autobiography disguised as fiction, in which the hero/heroine hides crucial intrapsychic conflicts, mysteries, screen memories of actual traumatic events and the resolution of these elements into a happy ending, best celebrated by orgasm. The function of the fantasy is to take these painful experiences and convert them to pleasure-triumph. In order to sharpen excitement-the vibration between the fear of original traumas repeating and the hope of a pleasurable conclusion this time-one introduces into the story elements of risk (approximations of the trauma) meant to prevent boredom and safety factors (sub-limnal signals to the storyteller that the risk are not truly dangerous). Sexual fantasy can be studied by means of a person's daydreams (including those chosen in magazines, books, plays, television, movies, and outright pornography), masturbatory behavior, object choice, foreplay, techniques of intercourse, or postcoital behavior. PMID:949223

  6. Modes of decay in neutron-rich nuclei

    NASA Astrophysics Data System (ADS)

    Kumar, B.; Biswal, S. K.; Singh, S. K.; Lahiri, C.; Patra, S. K.

    2016-03-01

    We calculate the ground, first intrinsic excited states and density distribution for neutron-rich thorium and uranium isotopes, within the framework of relativistic mean field (RMF) approach using axially deformed basis. The total nucleon densities are calculated, from which the cluster-structures inside the parent nuclei are determined. The possible modes of decay, like α-decay and β-decay are analyzed. We find the neutron-rich isotopes are stable against α-decay, however they are very much unstable against β-decay. The life time of these nuclei predicted to be tens of second against β-decay.

  7. {alpha} decay of high-spin isomers in superheavy nuclei

    SciTech Connect

    Delion, D. S.; Liotta, R. J.; Wyss, R.

    2007-10-15

    Hindrance factors corresponding to {alpha} decay from two quasiparticle isomeric high K states are evaluated in superheavy nuclei. We found that the hindrance factors are very sensitive to the deformations and, therefore, they may constitute a powerful tool to extract spectroscopic information in these nuclei. The hindrance factors turn out to be very large, specially for nonaligned configurations. This indicates that if one of such states is reached the parent nucleus may become isomeric. It is also possible that {alpha} decay may not proceed through ground state to ground state chains but rather through excited states.

  8. Shell Model Description of the Odd-Odd Co and Cu Nuclei

    SciTech Connect

    Medina, N. H.; Allegro, P. R. P.; Oliveira, J. R. B. de; Ribas, R. V.; Seale, W. A.; Toufen, D. L.; Silveira, M. A. G.

    2007-10-26

    The known excited states of the odd-odd nuclei {sup 54,56,58,60}Co and 60,62,64,66Cu were interpreted in the framework of the large scale shell model (LSSM), using several effective interactions and configuration spaces. For the description of the negative parity states, we have allowed one particle excitation to the g{sub 9/2} orbital. The LSSM using the GXPF1 effective interaction reproduces well the first excited states in all of these nuclei.

  9. Properties of Cometary Nuclei

    NASA Technical Reports Server (NTRS)

    Rahe, J.; Vanysek, V.; Weissman, P. R.

    1994-01-01

    Active long- and short-period comets contribute about 20 to 30 % of the major impactors on the Earth. Cometary nuclei are irregular bodies, typically a few to ten kilometers in diameter, with masses in the range 10(sup 15) to 10(sup 18) g. The nuclei are composed of an intimate mixture of volatile ices, mostly water ice and hydrocarbon and silicate grains. The composition is the closest to solar composition of any known bodies in the solar system. The nuclei appear to be weakly bonded agglomerations of smaller icy planetesimals, and material strengths estimated from observed tidal disruption events are fairly low, typically 10(sup 2) to 10(sup 4) N m(sup -2). Density estimates range between 0.2 and 1.2 g cm(sup -3) but are very poorly determined, if at all. As comets age they develop nonvolitile crusts on their surfaces which eventually render them inactive, similar in appearance to carbonaceous asteroids. However, dormant comets may continue to show sporadic activity and outbursts for some time before they become truly extinct. The source of the long-period comets is the Oort cloud, a vast spherical cloud of perhaps 10(sup 12) to 10(sup 13) comets surrounding the solar system and extending to interstellar distances. The likely source for short-period comets is the Kuiper belt. a ring of perhaps 10(sup 8) to 10(sup 10) remnant icy planetesimals beyond the orbit of Neptune, though some short-period comets may also be long-period comets from the Oort cloud which have been perturbed into short-period orbits.

  10. Decay of {sup 118,122}Ba* compound nuclei formed in {sup 78,82}Kr+{sup 40}Ca reactions using the dynamical cluster-decay model of preformed clusters

    SciTech Connect

    Kumar, Raj; Gupta, Raj K.

    2009-03-15

    Application of the preformed clusters based dynamical cluster-decay model (DCM) is made to the recent data on decay of the compound systems {sup 118,122}Ba* at a relatively low bombarding energy of 5.5 MeV/A. The same model has been applied earlier to the intermediate mass fragment (IMF) data of {sup 116}Ba*, observed at medium and higher incident energies. For the heavier {sup 118,122}Ba* systems, however, a complete mass fragmentation spectrum is observed experimentally. Except for a small narrow region of heavier mass fragments (8{<=}Z{sub L}{<=}15), the DCM gives an overall reasonable description of the observed data on both the intermediate mass fragments and the fusion-fission cross-sections, whereas the statistical model calculations based on BUSCO and GEMINI codes describe the intermediate mass fragment data and the heavier mass fragment and fusion-fission data, respectively. Within the DCM (with preformation factor P{sub 0}=1), the possibility of non-compound-nucleus decay contributing to the region 8{<=}Z{sub L}{<=}15 of heavier mass fragments is also explored. All three models use the maximum angular momentum l{sub max} as a fitting parameter, which in the DCM is fixed via a neck-length parameter for the penetrability P{yields}1.