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Sample records for high energy spin

  1. Spin structure in high energy processes: Proceedings

    SciTech Connect

    DePorcel, L.; Dunwoodie, C.

    1994-12-01

    This report contains papers as the following topics: Spin, Mass, and Symmetry; physics with polarized Z{sup 0}s; spin and precision electroweak physics; polarized electron sources; polarization phenomena in quantum chromodynamics; polarized lepton-nucleon scattering; polarized targets in high energy physics; spin dynamics in storage rings and linear accelerators; spin formalism and applications to new physics searches; precision electroweak physics at LEP; recent results on heavy flavor physics from LEP experiments using 1990--1992 data; precise measurement of the left-right cross section asymmetry in Z boson production by electron-positron collisions; preliminary results on heavy flavor physics at SLD; QCD tests with SLD and polarized beams; recent results from TRISTAN at KEK; recent B physics results from CLEO; searching for the H dibaryon at Brookhaven; recent results from the compton observatory; the spin structure of the deuteron; spin structure of the neutron ({sup 3}HE) and the Bjoerken sum rule; a consumer`s guide to lattice QCD results; top ten models constrained by b {yields} sy; a review of the Fermilab fixed target program; results from the D0 experiment; results from CDF at FNAL; quantum-mechanical suppression of bremsstrahlung; report from the ZEUS collaboration at HERA; physics from the first year of H1 at HERA, and hard diffraction. These papers have been cataloged separately elsewhere.

  2. Spin Effects in High Energy Fragmentation Processes

    NASA Astrophysics Data System (ADS)

    Liang, Zuo-Tang

    Recent measurements, in particular those on Λ polarization and spin alignment of vector mesons in e+e- annihilation at LEP, and those on the azimuthal asymmetry at HERA, have attracted much attention on the spin effects in high energy fragmentation processes. In this talk, we make a brief introduction to the different topics studied in this connection and a short summary of the available data. After that, we present a short summary of the main theoretical results that we obtained in studying these different topics. The talk was mainly based on the publications [5-9] which have been finished in collaboration with C.Boros, Liu Chun-xiu and Xu Qing-hua.

  3. High energy neutrino spin light [rapid communication

    NASA Astrophysics Data System (ADS)

    Lobanov, A. E.

    2005-07-01

    The quantum theory of spin light (electromagnetic radiation emitted by a Dirac massive neutrino propagating in dense matter due to the weak interaction of a neutrino with background fermions) is developed. In contrast to the Cherenkov radiation, this effect does not disappear even if the medium refractive index is assumed to be equal to unity. The formulas for the transition rate and the total radiation power are obtained. It is found out that radiation of photons is possible only when the sign of the particle helicity is opposite to that of the effective potential describing the interaction of a neutrino (antineutrino) with the background medium. Due to the radiative self-polarization the radiating particle can change its helicity. As a result, the active left-handed polarized neutrino (right-handed polarized antineutrino) converting to the state with inverse helicity can become practically "sterile". Since the sign of the effective potential depends on the neutrino flavor and the matter structure, the spin light can change a ratio of active neutrinos of different flavors. In the ultra relativistic approach, the radiated photons averaged energy is equal to one third of the initial neutrino energy, and two thirds of the energy are carried out by the final "sterile" neutrinos.

  4. Hadronization Mechanisms and Spin Effects in High Energy Fragmentation Processes

    NASA Astrophysics Data System (ADS)

    Liang, Zuo-Tang

    2002-03-01

    Spin effects in high energy fragmentation processes can provide us with important information on hadronization mechanisms and spin structure of hadrons. It can in particular give new tests to the hadronization models. In this talk, we make a brief introduction to the different topics studied in this connection and a short summary of the available data. After that, we present a short summary of the main theoretical results we obtained in studying these different topics. The talk was mainly based on the publications [4-8] which have been finished in collaboration with C.Boros, Liu Chun-xiu and Xu Qing-hua.

  5. XVI Workshop on High Energy Spin Physics (D-SPIN2015)

    NASA Astrophysics Data System (ADS)

    Lednicky, Richard

    2016-02-01

    Dear Colleagues, Ladies and Gentlemen, on behalf of the Directorate of Joint Institute for Nuclear Research (JINR) it is a pleasure for me to welcome you here to Dubna for the 16th International Workshop on High Energy Spin Physics. It provides an opportunity to present and discuss the news accumulated during last year. Another important feature of this series of workshops has always been the participation of a large number of physicists from the former Soviet Union and Eastern European countries, for which long trips have previously been limited by financial (and earlier also by bureaucratic) reasons. It thus represents an important addition to the series of large International Symposia on spin physics held in even-numbered years in different countries, including the Symposium held in Dubna in 2012. JINR has a long-lasting tradition of experimental and theoretical studies of spin phenomena. The workshops on high energy spin physics started in Dubna in 1981 due to the initiative of L. Lapidus, an outstanding theoretical physicist. Since then, these meetings have been held in Dubna in every odd year and have become regular thanks to Anatoly Vasilievich Efremov, the chairman for many years. Recent years have brought a lot of new experimental results, and above all the discovery and determination of quantum characteristics of the Higgs boson at the Large Hadron Collider.

  6. Summary of the 9th international symposium on high energy spin-physics

    SciTech Connect

    Prescott, C.Y.

    1990-11-01

    Summarizing an international conference in high energy spin physics is never an easy task, because of the wide-ranging subjects in physics and technology that are involved. I have chosen to organize the topics of this conference into three broad categories relating to spin; intrinsic spin; composite spin; and spin, the experimental tool. In the first category, I will briefly revisit some historical and recent developments to set a background. In the second category, composite spin, I will discuss the status and developments in several areas, including magnetic moments of baryons, hyperon polarization in high energy high p {perpendicular} production, transverse polarization and asymmetries from transversely polarized targets in high p {perpendicular} scattering, spin structure of the proton, and the Bjorken sum rule. In the third category, I will discuss the steady, and at times rapid, progress in spin technology. In this part I include recent progress in high energy facilities, and comment on the highlights of the Workshops.

  7. Design and performance of a spin-polarized electron energy loss spectrometer with high momentum resolution.

    PubMed

    Vasilyev, D; Kirschner, J

    2016-08-01

    We describe a new "complete" spin-polarized electron energy loss spectrometer comprising a spin-polarized primary electron source, an imaging electron analyzer, and a spin analyzer of the "spin-polarizing mirror" type. Unlike previous instruments, we have a high momentum resolution of less than 0.04 Å(-1), at an energy resolution of 90-130 meV. Unlike all previous studies which reported rather broad featureless data in both energy and angle dependence, we find richly structured spectra depending sensitively on small changes of the primary energy, the kinetic energy after scattering, and of the angle of incidence. The key factor is the momentum resolution. PMID:27587131

  8. Spin effects in high-energy photon-hadron scattering in QCD

    SciTech Connect

    Goloskokov, S.V.; Listopadov, O.A.

    1995-09-01

    Spin effects at high energies and momentum transfers {vert_bar}t{vert_bar} > 1 GeV{sup 2} are analyzed for elastic quark-photon scattering. The ratio of the spin-flip and non-spin-flip amplitudes in the same order of perturbative QCD is found to be independent of energy. It is shown that the contribution of the spin-dependent quark-pomeron vertex to the photon spin-flip amplitude is enhanced by off-mass-shell effects in the quark loop. As a result, this amplitude can become as large as 20-30% of the non-spin-flip amplitude. The cross section is found to depend on the form factor and on contributions of order {alpha}{sub s}{sup 3} the non-spin-flip amplitude. 12 refs., 4 figs.

  9. Analysis of possibilities for a spin flip in high energy electron ring HERA

    SciTech Connect

    Stres, S.; Pestotnik, R.

    2007-06-13

    In a high energy electron ring the spins of electrons become spontaneously polarized via the emission of spin-flip synchrotron radiation. By employing a radio frequency (RF) radial dipole field kicker, particle spin directions can be rotated slowly over many turns. A model which couples three dimensional spin motion and longitudinal particle motion was constructed to describe non-equilibrium spin dynamics in high energy electron storage rings. The effects of a stochastic synchrotron radiation on the orbital motion in the accelerator synchrotron plane and its influence on the spin motion are studied. The main contributions to the spin motion, the synchrotron oscillations and the stochastic synchrotron radiation, have different influence on the spin polarization reversal in different regions of the parameter space. The results indicate that polarization reversal might be obtained in high energy electron storage rings with a significant noise even with relatively small strengths of a perturbing magnetic field. The only experimental datum avaliable agrees with the model prediction, however further experimental data would be necessary to validate the model.

  10. High-order moments of spin-orbit energy in a multielectron configuration.

    PubMed

    Na, Xieyu; Poirier, M

    2016-07-01

    In order to analyze the energy-level distribution in complex ions such as those found in warm dense plasmas, this paper provides values for high-order moments of the spin-orbit energy in a multielectron configuration. Using second-quantization results and standard angular algebra or fully analytical expressions, explicit values are given for moments up to 10th order for the spin-orbit energy. Two analytical methods are proposed, using the uncoupled or coupled orbital and spin angular momenta. The case of multiple open subshells is considered with the help of cumulants. The proposed expressions for spin-orbit energy moments are compared to numerical computations from Cowan's code and agree with them. The convergence of the Gram-Charlier expansion involving these spin-orbit moments is analyzed. While a spectrum with infinitely thin components cannot be adequately represented by such an expansion, a suitable convolution procedure ensures the convergence of the Gram-Charlier series provided high-order terms are accounted for. A corrected analytical formula for the third-order moment involving both spin-orbit and electron-electron interactions turns out to be in fair agreement with Cowan's numerical computations. PMID:27575229

  11. High-order moments of spin-orbit energy in a multielectron configuration

    NASA Astrophysics Data System (ADS)

    Na, Xieyu; Poirier, M.

    2016-07-01

    In order to analyze the energy-level distribution in complex ions such as those found in warm dense plasmas, this paper provides values for high-order moments of the spin-orbit energy in a multielectron configuration. Using second-quantization results and standard angular algebra or fully analytical expressions, explicit values are given for moments up to 10th order for the spin-orbit energy. Two analytical methods are proposed, using the uncoupled or coupled orbital and spin angular momenta. The case of multiple open subshells is considered with the help of cumulants. The proposed expressions for spin-orbit energy moments are compared to numerical computations from Cowan's code and agree with them. The convergence of the Gram-Charlier expansion involving these spin-orbit moments is analyzed. While a spectrum with infinitely thin components cannot be adequately represented by such an expansion, a suitable convolution procedure ensures the convergence of the Gram-Charlier series provided high-order terms are accounted for. A corrected analytical formula for the third-order moment involving both spin-orbit and electron-electron interactions turns out to be in fair agreement with Cowan's numerical computations.

  12. Universality, maximum radiation, and absorption in high-energy collisions of black holes with spin.

    PubMed

    Sperhake, Ulrich; Berti, Emanuele; Cardoso, Vitor; Pretorius, Frans

    2013-07-26

    We explore the impact of black hole spins on the dynamics of high-energy black hole collisions. We report results from numerical simulations with γ factors up to 2.49 and dimensionless spin parameter χ=+0.85, +0.6, 0, -0.6, -0.85. We find that the scattering threshold becomes independent of spin at large center-of-mass energies, confirming previous conjectures that structure does not matter in ultrarelativistic collisions. It has further been argued that in this limit all of the kinetic energy of the system may be radiated by fine tuning the impact parameter to threshold. On the contrary, we find that only about 60% of the kinetic energy is radiated for γ=2.49. By monitoring apparent horizons before and after scattering events we show that the "missing energy" is absorbed by the individual black holes in the encounter, and moreover the individual black-hole spins change significantly. We support this conclusion with perturbative calculations. An extrapolation of our results to the limit γ→∞ suggests that about half of the center-of-mass energy of the system can be emitted in gravitational radiation, while the rest must be converted into rest-mass and spin energy. PMID:23931346

  13. Spin-spin correlations in proton-proton collisions at high energy and threshold enhancements

    SciTech Connect

    de Teramond, G.F.

    1988-05-01

    The striking effects in the spin structure observed in elastic proton collisions and the Nuclear Transparency phenomenon recently discovered at BNL are described in terms of heavy quark threshold enhancements. The deviations from scaling laws and the broadening of the angular distributions at resonance are also consistent with the introduction of new degrees of freedom in the pp system. This implies new s-channel physics. Predictions are given for the spin effects in pp collisions near 18.5 GeV/c at large p/sub T//sup 2/ where new measurements are planned. 9 refs., 4 figs.

  14. Dawn of High Energy Spin Physics — In Memory of Michel Borghini

    NASA Astrophysics Data System (ADS)

    Masaike, Akira

    2016-02-01

    High energy spin physics with the polarized proton target in 1960s is shown. The dynamic polarization in which the electronic polarization is transferred to protons in paramagnetic material by means of magnetic coupling was proposed at the beginning of 1960s. The first N-N experiment using a polarized proton target was performed with the crystal of La2Mg3 (NO3)1224H2O at CEN-Saclay and Berkeley in 1962, followed by π-p experiments in several laboratories. Protons in organic materials were found to be polarized up to 80% in 3He cryostats in 1969. It was helpful for large background experiments. High proton polarization was interpreted in the spin temperature theory. Spin frozen targets were constructed in early 1970s and used for experiments which require wide access angle. Michel Borghini was a main player for almost all the above works.

  15. PROCEEDINGS OF RIKEN BNL RESEARCH CENTER WORKSHOP CIRCUM-PAN-PACIFIC RIKEN SYMPOSIUM ON HIGH ENERGY SPIN PHYSICS, VOLUME 25

    SciTech Connect

    KUMANO,S.; SHIBATA,T.A.; YAZAKI,K.

    2000-06-28

    The Circum-Pan-Pacific Riken Symposium on High Energy Spin Physics was held at Oukouchi Memorial Hall in Riken from November 3 through 6, 1999. It was held as a joint meeting of the 2nd Circum-Pan-Pacific Symposium on High Energy Spin Physics and the 3rd of the series of Riken Symposia related to the RHIC-SPIN. The 1st Circum-Pan-Pacific Symposium on High Energy Spin Physics was held at Kobe in 1996 and the RHIC-SPIN Riken Symposia had been held every two years since 1995. As Prof. Ozaki mentioned in his talk at the beginning of this meeting, the RHIC was ready for the first beam, physics experiments scheduled in 2000, and the RHIC-SPIN would start in 2001. It was therefore considered to be very timely for the researchers in the field of high energy spin physics to get together, clarifying the present status of the field and discussing interesting and important topics as well as experimental subjects to be pursued. It is especially important for the success of the RHIC-SPIN project that the researchers in the neighboring countries surrounding the Pacific are actively involved in it. This is why the above two series were joined in this. symposium. The subjects discussed in the symposium include: Hard processes probing spin-structure functions, polarization mechanisms in high energy reactions, lattice studies of polarized structure functions, theoretical models for the nucleon and its spin structure, RHIC and RHIC-SPIN projects, results and future projects of existing experimental facilities. Totally 73 scientists participated in the symposium, 27 from abroad and 46 from Japan. it consisted of 13 main sessions, with 33 invited and contributed talks, and 4 discussion sessions covering recent experimental and theoretical developments and important topics in high energy spin physics and closely related fields.

  16. Internal spin structure of the proton from high energy polarized e-p scattering

    SciTech Connect

    Hughes, V.W.; Baum, G.; Bergstroem, M.R.

    1981-02-01

    A review is given of experimental knowledge of the spin dependent structure functions of the proton, which is based on inclusive high energy scattering of longitudinal polarized electrons by longitudinally polarized protons in both the deep inelastic and resonance regions, and includes preliminary results from our most recent SLAC experiment. Implications for scaling, sum rules, models of proton structure, and the hyperfine structure interval in hydrogen are given. Possible future directions of research are indicated.

  17. Pairing Correlations at High Spins

    NASA Astrophysics Data System (ADS)

    Ma, Hai-Liang; Dong, Bao-Guo; Zhang, Yan; Fan, Ping; Yuan, Da-Qing; Zhu, Shen-Yun; Zhang, Huan-Qiao; Petrache, C. M.; Ragnarsson, I.; Carlsson, B. G.

    The pairing correcting energies at high spins in 161Lu and 138Nd are studied by comparing the results of the cranked-Nilsson-Strutinsky (CNS) and cranked-Nilsson-Strutinsky-Bogoliubov (CNSB) models. It is concluded that the Coriolis effect rather than the rotational alignment effect plays a major role in the reduction of the pairing correlations in the high spin region. Then we proposed an average pairing correction method which not only better reproduces the experimental data comparing with the CNS model but also enables a clean-cut tracing of the configurations thus the full-spin-range discussion on the various rotating bands.

  18. Spin-Torque Sensors for Energy Efficient High-Speed Long Interconnects

    NASA Astrophysics Data System (ADS)

    Azim, Zubair Al; Sengupta, Abhronil; Sarwar, Syed Shakib; Roy, Kaushik

    2016-02-01

    In this paper, we propose a Spin-Torque (ST) based sensing scheme that can enable energy efficient multi-bit long distance interconnect architectures. Current-mode interconnects have recently been proposed to overcome the performance degradations associated with conventional voltage mode Copper (Cu) interconnects. However, the performance of current mode interconnects are limited by analog current sensing transceivers and equalization circuits. As a solution, we propose the use of ST based receivers that use Magnetic Tunnel Junctions (MTJ) and simple digital components for current-to-voltage conversion and do not require analog transceivers. We incorporate Spin-Hall Metal (SHM) in our design to achieve high speed sensing. We show both single and multi-bit operations that reveal major benefits at higher speeds. Our simulation results show that the proposed technique consumes only 3.93-4.72 fJ/bit/mm energy while operating at 1-2 Gbits/sec; which is considerably better than existing charge based interconnects. In addition, Voltage Controlled Magnetic Anisotropy (VCMA) can reduce the required current at the sensor. With the inclusion of VCMA, the energy consumption can be further reduced to 2.02-4.02 fJ/bit/mm

  19. High-energy spin-density-wave correlated fluctuations in paramagnetic Cr + 5 at. % V

    SciTech Connect

    Werner, S.A.; Fawcett, E.; Elmiger, M.W.; Shirane, G.

    1992-11-01

    Measurements of the magnetic fluctuations, termed spin-density-wave (SDW) paramagnons, in the nearly antiferromagnetic alloy Cr + 5 at.%V are extended up in energy to about 80 MeV. These fluctuating spin-spin correlations occur at incommensurate positions, corresponding to the SDW wavevector Q. Their characteristic energy is at least an order of magnitude larger than that of the magnetic fluctuations seen in the paramagnetic phase of pure Cr, but their intensity is more than two orders of magnitude smaller. We find that the dynamic susceptibility decreases by about 50% between temperature T = 10K and 300K.

  20. High-energy spin-density-wave correlated fluctuations in paramagnetic Cr + 5 at. % V

    SciTech Connect

    Werner, S.A. . Dept. of Physics); Fawcett, E. . Dept. of Physics); Elmiger, M.W.; Shirane, G. )

    1992-01-01

    Measurements of the magnetic fluctuations, termed spin-density-wave (SDW) paramagnons, in the nearly antiferromagnetic alloy Cr + 5 at.%V are extended up in energy to about 80 MeV. These fluctuating spin-spin correlations occur at incommensurate positions, corresponding to the SDW wavevector Q. Their characteristic energy is at least an order of magnitude larger than that of the magnetic fluctuations seen in the paramagnetic phase of pure Cr, but their intensity is more than two orders of magnitude smaller. We find that the dynamic susceptibility decreases by about 50% between temperature T = 10K and 300K.

  1. Highly efficient spin filtering of ballistic electrons

    NASA Astrophysics Data System (ADS)

    Steinmuller, S. J.; Trypiniotis, T.; Cho, W. S.; Hirohata, A.; Lew, W. S.; Vaz, C. A.; Bland, J. A.

    2004-04-01

    Spin dependent electron transport in hybrid Au/Co/Cu/NiFe/n-GaAs spin valve Schottky barrier structures was investigated using photoexcitation at various wavelengths. For excitation with the photon energy well above the Schottky barrier height we found a ˜2400% increase in helicity dependent photocurrent on switching the spin valve from parallel to antiparallel alignment. Our observations provide clear evidence for highly efficient spin filtering of spin polarized ballistic electrons.

  2. Spin-polarized high-energy scattering of charged leptons on nucleons

    SciTech Connect

    Burkardt, Matthias; Nowak, Wolf-Dieter; MILLER, A.

    2009-01-01

    The proton is a composite object with spin one-half, understood to contain highly relativistic spin one-half quarks exchanging spin-one gluons, each possibly with significant orbital angular momenta. While their fundamental interactions are well described by Quantum ChromoDynamics (QCD), our standard theory of the strong interaction, nonperturbative calculations of the internal structure of the proton based directly on QCD are beginning to provide reliable results. Most of our present knowledge of the structure of the proton is based on experimental measurements interpreted within the rich framework of QCD. An area presently attracting intense interest, both experimental and theoretical, is the relationship between the spin of the proton and the spins and orbital angular momenta of its constituents. While remarkable progress has been made, especially in the last decade, the discovery and investigation of new concepts have revealed that much more remains to be learned. This progress i

  3. Nuclear energy surfaces at high-spin in the A{approximately}180 mass region

    SciTech Connect

    Chasman, R.R.; Egido, J.L.; Robledo, L.M.

    1995-08-01

    We are studying nuclear energy surfaces at high spin, with an emphasis on very deformed shapes using two complementary methods: (1) the Strutinsky method for making surveys of mass regions and (2) Hartree-Fock calculations using a Gogny interaction to study specific nuclei that appear to be particularly interesting from the Strutinsky method calculations. The great advantage of the Strutinsky method is that one can study the energy surfaces of many nuclides ({approximately}300) with a single set of calculations. Although the Hartree-Fock calculations are quite time-consuming relative to the Strutinsky calculations, they determine the shape at a minimum without being limited to a few deformation modes. We completed a study of {sup 182}Os using both approaches. In our cranked Strutinsky calculations, which incorporate a necking mode deformation in addition to quadrupole and hexadecapole deformations, we found three well-separated, deep, strongly deformed minima. The first is characterized by nuclear shapes with axis ratios of 1.5:1; the second by axis ratios of 2.2:1 and the third by axis ratios of 2.9:1. We also studied this nuclide with the density-dependent Gogny interaction at I = 60 using the Hartree-Fock method and found minima characterized by shapes with axis ratios of 1.5:1 and 2.2:1. A comparison of the shapes at these minima, generated in the two calculations, shows that the necking mode of deformation is extremely useful for generating nuclear shapes at large deformation that minimize the energy. The Hartree-Fock calculations are being extended to larger deformations in order to further explore the energy surface in the region of the 2.9:1 minimum.

  4. Enhanced spin polarization in graphene with spin energy gap induced by spin-orbit coupling and strain

    SciTech Connect

    Liu, Zheng-Fang; Wu, Qing-Ping E-mail: aixichen@ecjtu.jx.cn; Chen, Ai-Xi E-mail: aixichen@ecjtu.jx.cn; Xiao, Xian-Bo; Liu, Nian-Hua

    2014-05-28

    We investigate the possibility of spin polarization in graphene. The result shows that a spin energy gap can be opened in the presence of both spin-orbit coupling and strain. We find that high spin polarization with large spin-polarized current is achieved in the spin energy gap. However, only one of the two modulations is present, no spin polarization can be generated. So the combination of the two modulations provides a way to design tunable spin polarization without need for a magnetic element or an external magnetic field.

  5. High spin isomer beam line at RIKEN

    SciTech Connect

    Kishida, T.; Ideguchi, E.; Wu, H.Y.

    1996-12-31

    Nuclear high spin states have been the subject of extensive experimental and theoretical studies. For the production of high spin states, fusion reactions are usually used. The orbital angular momentum brought in the reaction is changed into the nuclear spin of the compound nucleus. However, the maximum induced angular momentum is limited in this mechanism by the maximum impact parameter of the fusion reaction and by the competition with fission reactions. It is, therefore, difficult to populate very high spin states, and as a result, large {gamma}-detector arrays have been developed in order to detect subtle signals from such very high spin states. The use of high spin isomers in the fusion reactions can break this limitation because the high spin isomers have their intrinsic angular momentum, which can bring the additional angular momentum without increasing the excitation energy. There are two methods to use the high spin isomers for secondary reactions: the use of the high spin isomers as a target and that as a beam. A high spin isomer target has already been developed and used for several experiments. But this method has an inevitable shortcoming that only {open_quotes}long-lived{close_quotes} isomers can be used for a target: {sup 178}Hf{sup m2} (16{sup +}) with a half-life of 31 years in the present case. By developing a high spin isomer beam, the authors can utilize various short-lived isomers with a short half-life around 1 {mu}s. The high spin isomer beam line of RIKEN Accelerator Facility is a unique apparatus in the world which provides a high spin isomer as a secondary beam. The combination of fusion-evaporation reaction and inverse kinematics are used to produce high spin isomer beams; in particular, the adoption of `inverse kinematics` is essential to use short-lived isomers as a beam.

  6. Energy distributions at the high-spin ferric sites in myoglobin crystals.

    PubMed Central

    Fiamingo, F G; Brill, A S; Hampton, D A; Thorkildsen, R

    1989-01-01

    The orientation and temperature dependence (4.2-2.5 K) of electron paramagnetic resonance (EPR) power saturation and spin-lattice relaxation rate, and the orientation dependence of signal linewidth, were measured in single crystals of the aquo complex of ferric sperm whale skeletal muscle myoglobin. The spin-packet linewidth was found to be temperature independent and to vary by a factor of seven within the heme plane. An analysis is presented which enables one to arrive at (a) hyperfine component line-widths and, from the in-plane angular variation of the latter, at (b) the widths of distributions in energy differences between low-lying electronic levels and (c) the angular spread in the in-plane principal g-directions. The values of the energy level distributions in crystals obtained from the measurements and analysis reported here are compared with those obtained by a different method for the same protein complex in frozen solution. The spread in the rhombic energy splitting is significantly greater in solution than in the crystal. PMID:2539208

  7. High-energy damping by particle-hole excitations in the spin-wave spectrum of iron-based superconductors

    NASA Astrophysics Data System (ADS)

    Leong, Zhidong; Lee, Wei-Cheng; Lv, Weicheng; Phillips, Philip

    2014-09-01

    Using a degenerate double-exchange model, we investigate the spin excitation spectra of iron pnictides. The model consists of local spin moments on each Fe site, as well as itinerant electrons from the degenerate dxz and dyz orbitals. The local moments interact with each other through antiferromagnetic J1-J2 Heisenberg interactions, and they couple to the itinerant electrons through a ferromagnetic Hund coupling. We employ the fermionic spinon representation for the local moments and perform a generalized random-phase approximation calculation on both spinons and itinerant electrons. We find that in the (π ,0) magnetically ordered state, the spin-wave excitation at (π,π) is pushed to a higher energy due to the presence of itinerant electrons, which is consistent with a previous study using the Holstein-Primakoff transformation. In the paramagnetic state, the particle-hole continuum keeps the collective spin excitation near (π,π) at a higher energy even without any C4 symmetry breaking. The implications for recent high-temperature neutron scattering measurements will be discussed.

  8. High-Spin States in 124Ba

    NASA Astrophysics Data System (ADS)

    Al-Khatib, A.; Singh, A. K.; Huebel, H.; Bringel, P.; Buerger, A.; Neusser, A.; Schoenwasser, G.; Hagemann, G. B.; Hansen, C. R.; Herskind, B.; Sletten, G.; Algora, A.; Dombradi, Zs.; Gal, J.; Kalinka, G.; Molnar, J.; Nyako, B. M.; Sohler, D.; Timar, J.; Zolnai, L.; Kmiecik, M.; Maj, A.; Styczen, J.; Zuber, K.; Hauschild, K.; Korichi, A.; Lopez-Martens, A.; Roccaz, J.; Siem, S.; Hannachi, F.; Scheurer, J. N.; Bednarczyk, P.; Byrski, Th.; Curien, D.; Dorvaux, O.; Duchene, G.; Gall, B.; Khalfallah, F.; Piqueras, I.; Robin, J.; Juhasz, K.; Patel, S. B.; Evans, A. O.; Rainovski, G.; Airoldi, A.; Benzoni, G.; Bracco, A.; Camera, F.; Million, B.; Mason, P.; Paleni, A.; Sacchi, R.; Wieland, O.; Petrache, C. M.; Petrache, D.; La Rana, G.; Moro, R.; de Angelis, G.; Fallon, P.; Lee, I.-Y.; Lisle, J. C.; Cederwall, B.; Lagergren, K.; Lieder, R. M.; Podsvirova, E.; Gast, W.; Jaeger, H.; Redon, N.; Goergen, A.

    2005-04-01

    High-spin states in 124Ba were populated using the 64Ni(64Ni,4n)124Ba reaction at beam energies of 255 and 261 MeV. Gamma-ray coincidences were measured using the EUROBALL detector array.The charged-particle detector array DIAMANT provided channel selection. The previously known rotational bands are extended to higher spins. Five new bands are observed, one of them extends up to the spin 40 hbar region.

  9. Properties of nuclei at very high spin

    SciTech Connect

    Stephens, F.S.

    1980-09-01

    Nuclear structure at very high spins involves an interplay between collective (often rotational) and noncollective (individual particle alignment) behavior. The new techniques for studying ..gamma..-ray energy correlations promise to give detailed information about both of these aspects of nuclear behavior up to the very highest spins that can be populated. 17 figures.

  10. Mass Measurements and Implications for the Energy of the High-Spin Isomer in {sup 94}Ag

    SciTech Connect

    Kankainen, A.; Elomaa, V.-V.; Eronen, T.; Hager, U.; Hakala, J.; Jokinen, A.; Moore, I. D.; Penttilae, H.; Rahaman, S.; Rinta-Antila, S.; Rissanen, J.; Saastamoinen, A.; Sonoda, T.; Weber, C.; Aeystoe, J.; Batist, L.; Popov, A.; Seliverstov, D. M.; Eliseev, S.; Novikov, Yu. N.

    2008-10-03

    Nuclides in the vicinity of {sup 94}Ag have been studied with the Penning trap mass spectrometer JYFLTRAP at the Ion-Guide Isotope Separator On-Line. The masses of the two-proton-decay daughter {sup 92}Rh and the beta-decay daughter {sup 94}Pd of the high-spin isomer in {sup 94}Ag have been measured, and the masses of {sup 93}Pd and {sup 94}Ag have been deduced. When combined with the data from the one-proton- or two-proton-decay experiments, the results lead to contradictory mass excess values for the high-spin isomer in {sup 94}Ag, -46 370(170) or -44 970(100) keV, corresponding to excitation energies of 6960(400) or 8360(370) keV, respectively.

  11. Low energy nuclear spin excitations in Ho metal investigated by high resolution neutron spectroscopy.

    PubMed

    Chatterji, Tapan; Jalarvo, Niina

    2013-04-17

    We have investigated the low energy excitations in metallic Ho by high resolution neutron spectroscopy. We found at T = 3 K clear inelastic peaks in the energy loss and energy gain sides, along with the central elastic peak. The energy of this low energy excitation, which is 26.59 ± 0.02 μeV at T = 3 K, decreased continuously and became zero at TN ≈ 130 K. By fitting the data in the temperature range 100-127.5 K with a power law we obtained the power-law exponent β = 0.37 ± 0.02, which agrees with the expected value β = 0.367 for a three-dimensional Heisenberg model. Thus the energy of the low energy excitations can be associated with the order parameter. PMID:23507905

  12. Production cross sections for Lee-Wick massive electromagnetic bosons and for spin-zero and spin-one W bosons at high energies.

    NASA Technical Reports Server (NTRS)

    Linsker, R.

    1972-01-01

    Production cross sections for three types of hypothetical particles are calculated in the presented paper. Several (Z, Z') cases were studied corresponding to elastic scattering off protons and neutrons (either free or embedded within a Fermi sea), coherent scattering off a nucleus, and inelastic scattering off a proton (in which case Z' denotes a nucleon resonance or hadronic system in the continuum). Detailed structure-function data are used to improve the accuracy of the inelastic scattering calculation. Results of calculations are given for beam energies between 50 and 10,000 GeV, and masses between 5 and 40 GeV for the massive Lee-Wick spin-1 boson. Cross sections were computed for resonant and semiweak processes. The production cross section of spin-zero weak intermediate bosons was found to be at least one order of magnitude smaller than for spin-1 weak bosons in nearly all regions of interest. The production cross section of spin-zero weak intermediate bosons for inelastic scattering off protons compares with that for elastic scattering in the regions of interest. In the case of massive spin-1 bosons and spin-1 weak intermediates, the main contribution to total production cross section off protons is elastic.

  13. The Quest for Spinning Glue in High-Energy Polarized Proton-Proton Collisions at RHIC

    SciTech Connect

    Surrow, Bernd

    2007-10-26

    The STAR experiment at the Relativistic Heavy-Ion Collider (RHIC) at Brookhaven National Laboratory (BNL) is carrying out a spin physics program colliding transverse or longitudinal polarized proton beams at {radical}(s) = 200-500 GeV to gain a deeper insight into the spin structure and dynamics of the proton. These studies provide fundamental tests of Quantum Chromodynamics (QCD).One of the main objectives of the STAR spin physics program is the determination of the polarized gluon distribution function through a measurement of the longitudinal double-spin asymmetry, A{sub LL}, for various processes. Recent results will be shown on the measurement of A{sub LL} for inclusive jet production, neutral pion production and charged pion production at {radical}(s) = 200 GeV.

  14. Energy Transport in High-Density Spin-Exchange Optical Pumping Cells

    NASA Astrophysics Data System (ADS)

    Walter, D. K.; Griffith, W. M.; Happer, W.

    2001-04-01

    We present in situ measurements of temperatures inside multi-atmosphere spin-exchange optical pumping cells using Raman scattering from the N2 quenching gas. Under conditions usually prevailing in spin-exchange optical pumping experiments, we find that gas temperatures can be elevated hundreds of degrees above ambient, and that convection plays a very important role in the heat transport of the system.

  15. Magnetic-Field-Induced Low-Energy Spin Excitations in YBa2Cu4O8 Measured by High Field Gd3+ Electron Spin Resonance

    NASA Astrophysics Data System (ADS)

    Fehér, Titusz; Jánossy, András; Oszlányi, Gábor; Simon, Ferenc; Dabrowski, Bogdan; Klamut, Piotr W.; Horvatić, Mladen; Williams, Grant V.

    2000-12-01

    We have measured the spin susceptibility, χs, of the CuO2 planes in the underdoped high Tc superconductor, YBa2Cu4O8 by Gd3+ electron spin resonance (ESR) in single crystals and aligned powders in fields up to 15.4 T. At low temperatures and high fields, χs is enhanced slightly in the B∥c orientation with respect to the B⊥c orientation. The enhancement at 15.4 T ( ~0.15Hc2) at 16 K ( 0.2 Tc) is small: approximately 10% of χs\\(Tc\\), suggesting that the second critical field of superconductivity, Hc2~100 T, would not suppress the pseudogap. This work demonstrates the potential of high field ESR in single crystals for studying high Tc superconductors.

  16. Correlation Energy of 3D Spin-Polarized Electron Gas: A Single Interpolation Between High- and Low-Density Limits

    NASA Astrophysics Data System (ADS)

    Sun, Jianwei; Perdew, John; Seidl, Michael

    2008-03-01

    We present an analytic model for the correlation energy per electron ec(rs,ζ) in the three-dimensional (3D) uniform electron gas, covering the full range 0<=rs<∞ and 0<=ζ<=1 of the density parameter rs and the relative spin polarization ζ. An interpolation is made between the exactly known high-density (rs->0) and low-density (rs->∞) limits, using a formula which (unlike previous ones) has the right analytic structures in both limits. We find that there is almost enough information available from these limits to determine the correlation energy over the full range. By minimal fitting to numerical quantum Monte Carlo data, we predict the value of b1(ζ) at ζ=0 close to the theoretical value [1], where b1(ζ) is the coefficient of the rsterm in the high-density expansion. The model finds correlation energies for the unpolarized (ζ=0) and fully polarized (ζ=1) cases in excellent agreement with Monte Carlo data. [1] T. Endo, M. Horiuchi, Y. Takada and H. Yasuhara, Phys. Rev. B 59, 7367 (1999)

  17. High-Spin Cobalt Hydrides for Catalysis

    SciTech Connect

    Holland, Patrick L.

    2013-08-29

    Organometallic chemists have traditionally used catalysts with strong-field ligands that give low-spin complexes. However, complexes with a weak ligand field have weaker bonds and lower barriers to geometric changes, suggesting that they may lead to more rapid catalytic reactions. Developing our understanding of high-spin complexes requires the use of a broader range of spectroscopic techniques, but has the promise of changing the mechanism and/or selectivity of known catalytic reactions. These changes may enable the more efficient utilization of chemical resources. A special advantage of cobalt and iron catalysts is that the metals are more abundant and cheaper than those currently used for major industrial processes that convert unsaturated organic molecules and biofeedstocks into useful chemicals. This project specifically evaluated the potential of high-spin cobalt complexes for small-molecule reactions for bond rearrangement and cleavage reactions relevant to hydrocarbon transformations. We have learned that many of these reactions proceed through crossing to different spin states: for example, high-spin complexes can flip one electron spin to access a lower-energy reaction pathway for beta-hydride elimination. This reaction enables new, selective olefin isomerization catalysis. The high-spin cobalt complexes also cleave the C-O bond of CO2 and the C-F bonds of fluoroarenes. In each case, the detailed mechanism of the reaction has been determined. Importantly, we have discovered that the cobalt catalysts described here give distinctive selectivities that are better than known catalysts. These selectivities come from a synergy between supporting ligand design and electronic control of the spin-state crossing in the reactions.

  18. Recent Results on High-Energy Spin Phenomena of Gluons and Sea-Quarks in Polarized Proton-Proton Collisions at Rhic at Bnl

    NASA Astrophysics Data System (ADS)

    Surrow, Bernd

    2014-01-01

    The STAR experiment at the Relativistic Heavy-Ion Collider at Brookhaven National Laboratory is carrying out a spin physics program in high-energy polarized proton collisions at √ {s} = 200 GeV and √ {s} = 500 GeV to gain a deeper insight into the spin structure and dynamics of the proton. One of the main objectives of the spin physics program at RHIC is the precise determination of the polarized gluon distribution function. The STAR detector is well suited for the reconstruction of various final states involving jets, π0, π±, e± and γ, which allows to measure several different processes. Recent results suggest a gluon spin contribution to the proton spin at the same level as the quark spin contribution itself. The production of W bosons in polarized p+p collisions at √ {s} = 500 GeV opens a new era in the study of the spin-flavor structure of the proton. W-(+) bosons are produced in \\bar {u} + d (\\bar {d} + u) collisions and can be detected through their leptonic decays, e- + \\bar {ν }e (e++ν e), where only the respective charged lepton is measured. Results of W-(+) production suggest a large asymmetry between the polarization of anti-u and anti-d quarks.

  19. High-spin structure of 102Ru

    NASA Astrophysics Data System (ADS)

    Sohler, D.; Timár, J.; Rainovski, G.; Joshi, P.; Starosta, K.; Fossan, D. B.; Molnár, J.; Wadsworth, R.; Algora, A.; Bednarczyk, P.; Curien, D.; Dombrádi, Zs.; Duchene, G.; Gizon, A.; Gizon, J.; Jenkins, D. G.; Koike, T.; Krasznahorkay, A.; Paul, E. S.; Raddon, P. M.; Scheurer, J. N.; Simons, A. J.; Vaman, C.; Wilkinson, A. R.; Zolnai, L.

    2005-06-01

    High-spin states in the nucleus 102Ru have been investigated via the 96Zr(13C,α3n) reaction at beam energies of 51 and 58 MeV, using the euroball IV γ-ray spectrometer and the diamant charged particle array. Several new high-spin bands have been established. The ground-state band has been extended up to Ex~12 MeV with Iπ=(26+); the previously published negative-parity bands have been extended up to Ex~11 and ˜ 9 MeV with Iπ=(23-) and (20-), respectively. The deduced high-spin structure has been compared with Woods-Saxon total Routhian surface calculations and, on the basis of the measured Routhians, aligned angular momenta, and B(M1)/B(E2) ratios, νh11/2(g7/2,d5/2) configurations are suggested for the negative-parity structures.

  20. High spin spectroscopy near the N=Z line: Channel selection and excitation energy systematics

    SciTech Connect

    Svensson, C.E.; Cameron, J.A.; Flibotte, S.

    1996-12-31

    The total {gamma}-ray and charged-particle energies emitted in fusion-evaporation reactions leading to N=Z compound systems in the A = 50-70 mass region have been measured with the 8{pi} {gamma}-ray spectrometer and the miniball charged-particle detector array. A new method of channel selection has been developed which combines particle identification with these total energy measurements and greatly improves upon the selectivity possible with particle detection alone. In addition, the event by event measurement of total {gamma}-ray energies using the BGO ball of the 8{pi} spectrometer has allowed a determination of excitation energies following particle evaporation for a large number of channels in several different reactions. The new channel selection procedure and excitation energy systematics are illustrated with data from the reaction of {sup 24}Mg on {sup 40}Ca at E{sub lab} = 80MeV.

  1. (A neutron scattering experiment to study the high-energy spin dynamics of the itinerant antiferromagnet Mn sub 90 Cu sub 10 )

    SciTech Connect

    Fernandez-Baca, J.A.

    1990-10-26

    The traveler performed a neutron scattering experiment to study the high-energy spin dynamics of the itinerant antiferromagnet. This experiment was conducted at a unique instrument located at the hot-neutron source at the ILL. The traveler also held various scientific discussions with ILL research staff members and visiting scientists.

  2. High spin states in {sup 139}Pm

    SciTech Connect

    Dhal, A.; Sinha, R. K.; Chaturvedi, L.; Agarwal, P.; Kumar, S.; Jain, A. K.; Kumar, R.; Govil, I. M.; Mukhopadhyay, S.; Chakraborty, A.; Krishichayan; Ray, S.; Ghugre, S. S.; Sinha, A. K.; Kumar, R.; Singh, R. P.; Muralithar, S.; Bhowmik, R. K.; Pancholi, S. C.; Gupta, J. B.

    2009-07-15

    The odd mass nucleus {sup 139}Pm has been studied to high spins through the {sup 116}Cd({sup 27}Al,4n){sup 139}Pm reaction at an incident beam energy of 120 MeV. The de-exciting {gamma}-rays were detected using an array of 12 Compton suppressed Ge detectors. A total of 46 new levels have been proposed in the present work as a result of the observation of 60 new {gamma}-rays. Four new bands including a {delta}J=1 sequence have been identified and all the earlier reported bands, other than the yrast band, have been extended to higher spins and excitation energy. The spin assignments for most of the newly reported levels have been made using the observed coincidence angular anisotropy. Tilted axis cranking calculations support the interpretation of two of the observed magnetic dipole sequences as examples of magnetic rotational bands.

  3. High-spin nuclear spectroscopy

    SciTech Connect

    Diamond, R.M.

    1986-07-01

    High-spin spectroscopy is the study of the changes in nuclear structure, properties, and behavior with increasing angular momentum. It involves the complex interplay between collective and single-particle motion, between shape and deformation changes, particle alignments, and changes in the pairing correlations. A review of progress in theory, experimentation, and instrumentation in this field is given. (DWL)

  4. High-spin states in ^88Kr

    NASA Astrophysics Data System (ADS)

    Fotiades, N.; Lisetskiy, A. F.; Cizewski, J. A.; Krücken, R.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Becker, J. A.; Younes, W.

    2007-10-01

    High-spin states in ^88Kr have been studied following the fission of the ^226Th compound nucleus formed in a fusion-evaporation reaction (^18O at 91 MeV on ^208Pb). The Gammasphere array was used to detect γ-ray coincidences. High-spin states up to spin (14^+) and ˜8 MeV excitation energy have been established. The level scheme reported for ^88Kr in the spontaneous fission of ^248Cm [1] has been enriched and extended to higher spin and excitation energies. Differences between the level scheme reported in [1] and that obtained in the present work will be discussed. The observed experimental states are also compared with theoretical shell-model and interacting-boson-model-2 calculations. This work has been supported by the U.S. Department of Energy under Contracts No. DE-AC52-06NA25396 (LANL), W-7405-ENG-48 (LLNL) and AC03-76SF00098 (LBNL) and by the National Science Foundation (Rutgers). [1] T. Rzaca-Urban et al., Eur. Phys. J. A 9, 165 (2000).

  5. High-spin structure in 40K

    NASA Astrophysics Data System (ADS)

    Söderström, P.-A.; Recchia, F.; Nyberg, J.; Gadea, A.; Lenzi, S. M.; Poves, A.; Ataç, A.; Aydin, S.; Bazzacco, D.; Bednarczyk, P.; Bellato, M.; Birkenbach, B.; Bortolato, D.; Boston, A. J.; Boston, H. C.; Bruyneel, B.; Bucurescu, D.; Calore, E.; Cederwall, B.; Charles, L.; Chavas, J.; Colosimo, S.; Crespi, F. C. L.; Cullen, D. M.; de Angelis, G.; Désesquelles, P.; Dosme, N.; Duchêne, G.; Eberth, J.; Farnea, E.; Filmer, F.; Görgen, A.; Gottardo, A.; Grębosz, J.; Gulmini, M.; Hess, H.; Hughes, T. A.; Jaworski, G.; Jolie, J.; Joshi, P.; Judson, D. S.; Jungclaus, A.; Karkour, N.; Karolak, M.; Kempley, R. S.; Khaplanov, A.; Korten, W.; Ljungvall, J.; Lunardi, S.; Maj, A.; Maron, G.; Męczyński, W.; Menegazzo, R.; Mengoni, D.; Michelagnoli, C.; Molini, P.; Napoli, D. R.; Nolan, P. J.; Norman, M.; Obertelli, A.; Podolyak, Zs.; Pullia, A.; Quintana, B.; Redon, N.; Regan, P. H.; Reiter, P.; Robinson, A. P.; Şahin, E.; Simpson, J.; Salsac, M. D.; Smith, J. F.; Stézowski, O.; Theisen, Ch.; Tonev, D.; Unsworth, C.; Ur, C. A.; Valiente-Dobón, J. J.; Wiens, A.

    2012-11-01

    High-spin states of 40K have been populated in the fusion-evaporation reaction 12C(30Si,np)40K and studied by means of γ-ray spectroscopy techniques using one triple-cluster detector of the Advanced Gamma Tracking Array at the Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali di Legnaro. Several states with excitation energy up to 8 MeV and spin up to 10- have been discovered. These states are discussed in terms of J=3 and T=0 neutron-proton hole pairs. Shell-model calculations in a large model space have shown good agreement with the experimental data for most of the energy levels. The evolution of the structure of this nucleus is here studied as a function of excitation energy and angular momentum.

  6. Anomalous High-Energy Waterfall-Like Electronic Structure in 5 d Transition Metal Oxide Sr2IrO4 with a Strong Spin-Orbit Coupling

    PubMed Central

    Liu, Yan; Yu, Li; Jia, Xiaowen; Zhao, Jianzhou; Weng, Hongming; Peng, Yingying; Chen, Chaoyu; Xie, Zhuojin; Mou, Daixiang; He, Junfeng; Liu, Xu; Feng, Ya; Yi, Hemian; Zhao, Lin; Liu, Guodong; He, Shaolong; Dong, Xiaoli; Zhang, Jun; Xu, Zuyan; Chen, Chuangtian; Cao, Gang; Dai, Xi; Fang, Zhong; Zhou, X. J.

    2015-01-01

    The low energy electronic structure of Sr2IrO4 has been well studied and understood in terms of an effective Jeff = 1/2 Mott insulator model. However, little work has been done in studying its high energy electronic behaviors. Here we report a new observation of the anomalous high energy electronic structure in Sr2IrO4. By taking high-resolution angle-resolved photoemission measurements on Sr2IrO4 over a wide energy range, we have revealed for the first time that the high energy electronic structures show unusual nearly-vertical bands that extend over a large energy range. Such anomalous high energy behaviors resemble the high energy waterfall features observed in the cuprate superconductors. While strong electron correlation plays an important role in producing high energy waterfall features in the cuprate superconductors, the revelation of the high energy anomalies in Sr2IrO4, which exhibits strong spin-orbit coupling and a moderate electron correlation, points to an unknown and novel route in generating exotic electronic excitations. PMID:26267653

  7. Anomalous High-Energy Waterfall-Like Electronic Structure in 5 d Transition Metal Oxide Sr2IrO4 with a Strong Spin-Orbit Coupling.

    PubMed

    Liu, Yan; Yu, Li; Jia, Xiaowen; Zhao, Jianzhou; Weng, Hongming; Peng, Yingying; Chen, Chaoyu; Xie, Zhuojin; Mou, Daixiang; He, Junfeng; Liu, Xu; Feng, Ya; Yi, Hemian; Zhao, Lin; Liu, Guodong; He, Shaolong; Dong, Xiaoli; Zhang, Jun; Xu, Zuyan; Chen, Chuangtian; Cao, Gang; Dai, Xi; Fang, Zhong; Zhou, X J

    2015-01-01

    The low energy electronic structure of Sr2IrO4 has been well studied and understood in terms of an effective Jeff = 1/2 Mott insulator model. However, little work has been done in studying its high energy electronic behaviors. Here we report a new observation of the anomalous high energy electronic structure in Sr2IrO4. By taking high-resolution angle-resolved photoemission measurements on Sr2IrO4 over a wide energy range, we have revealed for the first time that the high energy electronic structures show unusual nearly-vertical bands that extend over a large energy range. Such anomalous high energy behaviors resemble the high energy waterfall features observed in the cuprate superconductors. While strong electron correlation plays an important role in producing high energy waterfall features in the cuprate superconductors, the revelation of the high energy anomalies in Sr2IrO4, which exhibits strong spin-orbit coupling and a moderate electron correlation, points to an unknown and novel route in generating exotic electronic excitations. PMID:26267653

  8. Anomalous High-Energy Waterfall-Like Electronic Structure in 5 d Transition Metal Oxide Sr2IrO4 with a Strong Spin-Orbit Coupling

    NASA Astrophysics Data System (ADS)

    Liu, Yan; Yu, Li; Jia, Xiaowen; Zhao, Jianzhou; Weng, Hongming; Peng, Yingying; Chen, Chaoyu; Xie, Zhuojin; Mou, Daixiang; He, Junfeng; Liu, Xu; Feng, Ya; Yi, Hemian; Zhao, Lin; Liu, Guodong; He, Shaolong; Dong, Xiaoli; Zhang, Jun; Xu, Zuyan; Chen, Chuangtian; Cao, Gang; Dai, Xi; Fang, Zhong; Zhou, X. J.

    2015-08-01

    The low energy electronic structure of Sr2IrO4 has been well studied and understood in terms of an effective Jeff = 1/2 Mott insulator model. However, little work has been done in studying its high energy electronic behaviors. Here we report a new observation of the anomalous high energy electronic structure in Sr2IrO4. By taking high-resolution angle-resolved photoemission measurements on Sr2IrO4 over a wide energy range, we have revealed for the first time that the high energy electronic structures show unusual nearly-vertical bands that extend over a large energy range. Such anomalous high energy behaviors resemble the high energy waterfall features observed in the cuprate superconductors. While strong electron correlation plays an important role in producing high energy waterfall features in the cuprate superconductors, the revelation of the high energy anomalies in Sr2IrO4, which exhibits strong spin-orbit coupling and a moderate electron correlation, points to an unknown and novel route in generating exotic electronic excitations.

  9. High-spin structure of 134Xe

    NASA Astrophysics Data System (ADS)

    Vogt, A.; Birkenbach, B.; Reiter, P.; Blazhev, A.; Siciliano, M.; Valiente-Dobón, J. J.; Wheldon, C.; Bazzacco, D.; Bowry, M.; Bracco, A.; Bruyneel, B.; Chakrawarthy, R. S.; Chapman, R.; Cline, D.; Corradi, L.; Crespi, F. C. L.; Cromaz, M.; de Angelis, G.; Eberth, J.; Fallon, P.; Farnea, E.; Fioretto, E.; Freeman, S. J.; Gadea, A.; Geibel, K.; Gelletly, W.; Gengelbach, A.; Giaz, A.; Görgen, A.; Gottardo, A.; Hayes, A. B.; Hess, H.; Hua, H.; John, P. R.; Jolie, J.; Jungclaus, A.; Korten, W.; Lee, I. Y.; Leoni, S.; Liang, X.; Lunardi, S.; Macchiavelli, A. O.; Menegazzo, R.; Mengoni, D.; Michelagnoli, C.; Mijatović, T.; Montagnoli, G.; Montanari, D.; Napoli, D.; Pearson, C. J.; Pellegri, L.; Podolyák, Zs.; Pollarolo, G.; Pullia, A.; Radeck, F.; Recchia, F.; Regan, P. H.; Şahin, E.; Scarlassara, F.; Sletten, G.; Smith, J. F.; Söderström, P.-A.; Stefanini, A. M.; Steinbach, T.; Stezowski, O.; Szilner, S.; Szpak, B.; Teng, R.; Ur, C.; Vandone, V.; Ward, D.; Warner, D. D.; Wiens, A.; Wu, C. Y.

    2016-05-01

    Detailed spectroscopic information on the N ˜82 nuclei is necessary to benchmark shell-model calculations in the region. The nuclear structure above long-lived isomers in 134Xe is investigated after multinucleon transfer (MNT) and actinide fission. Xenon-134 was populated as (i) a transfer product in 238U+ 136Xe and 208Pb+ 136Xe MNT reactions and (ii) as a fission product in the 238U+ 136Xe reaction employing the high-resolution Advanced Gamma Tracking Array (AGATA). Trajectory reconstruction has been applied for the complete identification of beamlike transfer products with the magnetic spectrometer PRISMA. The 198Pt 136Xe MNT reaction was studied with the γ -ray spectrometer GAMMASPHERE in combination with the gas detector array Compact Heavy Ion Counter (CHICO). Several high-spin states in 134Xe on top of the two long-lived isomers are discovered based on γ γ -coincidence relationships and information on the γ -ray angular distributions as well as excitation energies from the total kinetic energy loss and fission fragments. The revised level scheme of 134Xe is extended up to an excitation energy of 5.832 MeV with tentative spin-parity assignments up to 16+. Previous assignments of states above the 7- isomer are revised. Latest shell-model calculations employing two different effective interactions reproduce the experimental findings and support the new spin and parity assignments.

  10. A revolutionary rotatable electron energy analyzer for advanced high-resolution spin-polarized photoemission studies. Final Report

    SciTech Connect

    Waddill, G. D.; Willis, R. F.

    1999-10-01

    This report details the construction and testing of a unique analyzer for spin-polarized photoemission studies of magnetic materials. This report details the progress of this project for the period from 9/1/96 through 8/31/99. Progress can be divided into two distinct areas. These are the fabrication, construction, and initial testing of the instrumentation, and the concurrent program of preliminary investigations into materials and experiments appropriate for future studies using the instrumentation developed. The analyzer complete with special input electron optics and Mott detector has been assembled in a special design UHV chamber equipped with all the capabilities needed to perform the described programs of research. These include a sophisticated five motorized axis sample manipulator with low and high temperature capability and rapid temperature cycling (acquired in collaboration with Dr. J.G. Tobin of LLNL), vacuum leak detection and gauging, in situ thin film growth instrumentation, and sample cleaning and magnetizing capabilities, The initial testing of the analyzer has been completed with successful data acquisition using both the multichannel detector mode, and spin-dependent using the Mott detector channeltrons. The data collected using the Mott detector were not truly spin dependent (see below), but demonstrate the operation of the lens and detector design. Acquisition of truly spin-dependent data await use of the EPU. Preliminary indications suggest that the analyzer performs at or above the original design parameters. In the second area of progress, we have conducted a number of preliminary studies toward the ends of identifying appropriate initial systems for investigation, and to further explore new experiments that the new instrumentation will help to pioneer. More detailed descriptions of all of these advances are given.

  11. High-spin structure of 104Pd

    NASA Astrophysics Data System (ADS)

    Sohler, D.; Kuti, I.; Timár, J.; Joshi, P.; Molnár, J.; Paul, E. S.; Starosta, K.; Wadsworth, R.; Algora, A.; Bednarczyk, P.; Curien, D.; Dombrádi, Zs.; Duchene, G.; Fossan, D. B.; Gál, J.; Gizon, A.; Gizon, J.; Jenkins, D. G.; Juhász, K.; Kalinka, G.; Koike, T.; Krasznahorkay, A.; Nyakó, B. M.; Raddon, P. M.; Rainovski, G.; Scheurer, J. N.; Simons, A. J.; Vaman, C.; Wilkinson, A. R.; Zolnai, L.

    2012-04-01

    The high-spin structure of the nucleus 104Pd was studied through the 96Zr(13C,5n) reaction at incident energies of 51 and 58 MeV, using the Euroball IV γ-ray spectrometer in conjunction with the DIAMANT charged-particle array. Several new medium- and high-spin bands were revealed. The already known positive-parity yrast and the negative-parity cascades were extended up to Ex˜13, ˜11, and ˜9 MeV with Iπ=(26+), Iπ=(23-), and (20-), respectively. The deduced band structures were compared with Woods-Saxon total Routhian surface (TRS) calculations. In addition, non-yrast low-lying positive-parity bands were identified, which were assigned to soft γ-vibrational excitations.

  12. Highly efficient spin-conversion effect leading to energy up-converted electroluminescence in singlet fission photovoltaics.

    PubMed

    Pandey, Ajay K

    2015-01-01

    Free charge generation in donor-acceptor (D-A) based organic photovoltaic diodes (OPV) progresses through formation of charge-transfer (CT) and charge-separated (CS) states and excitation decay to the triplet level is considered as a terminal loss. On the other hand a direct excitation decay to the triplet state is beneficial for multiexciton harvesting in singlet fission photovoltaics (SF-PV) and the formation of CT-state is considered as a limiting factor for multiple triplet harvesting. These two extremes when present in a D-A system are expected to provide important insights into the mechanism of free charge generation and spin-character of bimolecular recombination in OPVs. Herein, we present the complete cycle of events linked to spin conversion in the model OPV system of rubrene/C60. By tracking the spectral evolution of photocurrent generation at short-circuit and close to open-circuit conditions we are able to capture spectral changes to photocurrent that reveal the triplet character of CT-state. Furthermore, we unveil an energy up-conversion effect that sets in as a consequence of triplet population build-up where triplet-triplet annihilation (TTA) process effectively regenerates the singlet excitation. This detailed balance is shown to enable a rare event of photon emission just above the open-circuit voltage (V(OC)) in OPVs. PMID:25585937

  13. Highly efficient spin-conversion effect leading to energy up-converted electroluminescence in singlet fission photovoltaics

    NASA Astrophysics Data System (ADS)

    Pandey, Ajay K.

    2015-01-01

    Free charge generation in donor-acceptor (D-A) based organic photovoltaic diodes (OPV) progresses through formation of charge-transfer (CT) and charge-separated (CS) states and excitation decay to the triplet level is considered as a terminal loss. On the other hand a direct excitation decay to the triplet state is beneficial for multiexciton harvesting in singlet fission photovoltaics (SF-PV) and the formation of CT-state is considered as a limiting factor for multiple triplet harvesting. These two extremes when present in a D-A system are expected to provide important insights into the mechanism of free charge generation and spin-character of bimolecular recombination in OPVs. Herein, we present the complete cycle of events linked to spin conversion in the model OPV system of rubrene/C60. By tracking the spectral evolution of photocurrent generation at short-circuit and close to open-circuit conditions we are able to capture spectral changes to photocurrent that reveal the triplet character of CT-state. Furthermore, we unveil an energy up-conversion effect that sets in as a consequence of triplet population build-up where triplet-triplet annihilation (TTA) process effectively regenerates the singlet excitation. This detailed balance is shown to enable a rare event of photon emission just above the open-circuit voltage (VOC) in OPVs.

  14. Highly efficient spin-conversion effect leading to energy up-converted electroluminescence in singlet fission photovoltaics

    PubMed Central

    Pandey, Ajay K.

    2015-01-01

    Free charge generation in donor-acceptor (D-A) based organic photovoltaic diodes (OPV) progresses through formation of charge-transfer (CT) and charge-separated (CS) states and excitation decay to the triplet level is considered as a terminal loss. On the other hand a direct excitation decay to the triplet state is beneficial for multiexciton harvesting in singlet fission photovoltaics (SF-PV) and the formation of CT-state is considered as a limiting factor for multiple triplet harvesting. These two extremes when present in a D-A system are expected to provide important insights into the mechanism of free charge generation and spin-character of bimolecular recombination in OPVs. Herein, we present the complete cycle of events linked to spin conversion in the model OPV system of rubrene/C60. By tracking the spectral evolution of photocurrent generation at short-circuit and close to open-circuit conditions we are able to capture spectral changes to photocurrent that reveal the triplet character of CT-state. Furthermore, we unveil an energy up-conversion effect that sets in as a consequence of triplet population build-up where triplet-triplet annihilation (TTA) process effectively regenerates the singlet excitation. This detailed balance is shown to enable a rare event of photon emission just above the open-circuit voltage (VOC) in OPVs. PMID:25585937

  15. Direct observation of low energy nuclear spin excitations in HoCrO3 by high resolution neutron spectroscopy.

    PubMed

    Chatterji, T; Jalarvo, N; Kumar, C M N; Xiao, Y; Brückel, Th

    2013-07-17

    We have investigated low energy nuclear spin excitations in the strongly correlated electron compound HoCrO3. We observe clear inelastic peaks at E = 22.18 ± 0.04 μeV in both energy loss and gain sides. The energy of the inelastic peaks remains constant in the temperature range 1.5-40 K at which they are observed. The intensity of the inelastic peak increases at first with increasing temperature and then decreases at higher temperatures. The temperature dependence of the energy and intensity of the inelastic peaks is very unusual compared to that observed in other Nd, Co, V and also simple Ho compounds. Huge quasielastic scattering appears at higher temperatures presumably due to the fluctuating electronic moments of the Ho ions that get increasingly disordered at higher temperatures. The strong quasielastic scattering may also originate in the first Ho crystal-field excitations at about 1.5 meV. PMID:23779198

  16. Nuclear moments of inertia at high spins

    SciTech Connect

    Deleplanque, M.A.

    1983-12-01

    Nuclei with highest angular momentum are discussed. The production of high spin states, and the basic ideas associated with high spin physics are reviewed. Recent developments from continuum ..gamma..-ray studies are presented: the measurement of different average moments of inertia gives new information on the interplay between collective and single particle aspects at high spins. Finally, the exciting possibility of resolving the continuum spectra with new detector systems is examined. 8 references.

  17. A high-spin organic diradical as a spin filter.

    PubMed

    Shil, Suranjan; Bhattacharya, Debojit; Misra, Anirban; Klein, Douglas J

    2015-09-28

    Here, in this work we have designed a molecular bridge structure which can be used as a spin filter where the prototypical highly ferromagnetic m-phenylene connected bis(aminoxyl) diradical is used as a bridging fragment between two semi-infinitely widened gold (Au) electrodes along the [100] direction. A state-of-the-art non-equilibrium Green function's (NEGF) method coupled with the density functional theory (DFT) was carried out on this two-probe molecular bridge system to understand its electrical spin transport characteristics. The spin current at various bias voltages from 0.00 V to 4.00 V at intervals of 0.20 V for this Au-diradical-Au molecular junction is evaluated. We also quantify the bias-dependent spin injection coefficients (BDSIC) at different bias voltages and also the spin-filter efficiency at equilibrium, i.e., at zero bias voltage. Also plots of BDSIC vs. voltage, the up- and down-spin current vs. voltage (I-V) curves, and density of states (DOS) at zero bias voltage are evaluated. PMID:26287641

  18. High-Spin Gamma-Ray Spectroscopy in BISMUTH-198, Superdeformation in GOLD-191, and Multi-Photon Resonances in Low Energy Positron-Electron Scattering

    NASA Astrophysics Data System (ADS)

    Vo, Duc Ta.

    1993-01-01

    The properties of low-and high-spin levels in ^{198}Bi have been studied with the ^{181}Ta(^ {22}Ne,5n)^{198}Bi reaction at 116 MeV and 120 MeV bombarding energies. Levels along and near the yrast lines, including one isomer, were established up to spin J ~ 30hbar. The main configurations of these states are suggested to be pi h_{9/2} coupled to the known excited states in ^{197 }Pb. A sequence of states built on the excitation of the odd proton (coupled to one, two, or three quasi neutron-holes) was observed. In addition, at least two collective bands were observed. These two bands are backbending bands and are suggested to be oblate collective structures built on oblate proton and possibly neutron states. A superdeformed (SD) band was observed for the first time in an Au isotope. The reaction used was ^{11}B + ^{186 }W, demonstrating that very light ions can be used to populate SD bands at high angular momentum. The band is assigned to ^{191}Au. The gamma-ray energies are at the so -called quarter-point energies of the ^{192 }Hg SD band, indicating that the ^ {191}Au SD band is "identical" to that of ^{192}Hg. A search for resonant states in low-energy e ^+e^- scattering through their decay to multi-photon final states was performed using e ^+ from ^{68}Ga sources and a Pb absorber. Energy-sum and invariant mass spectra of coincident 2gamma and 3gamma events were obtained using the 20-element High Energy-Resolution Array (HERA) facility. No evidence for resonant states was found, and upper limits for the partial decay widths of such resonances were established in the energy range from 1.1 to 1.8 MeV.

  19. High Spin-Chern Insulators with Magnetic Order

    PubMed Central

    Ezawa, Motohiko

    2013-01-01

    As a topological insulator, the quantum Hall (QH) effect is indexed by the Chern and spin-Chern numbers and . We have only in conventional QH systems. We investigate QH effects in generic monolayer honeycomb systems. We search for spin-resolved characteristic patterns by exploring Hofstadter's butterfly diagrams in the lattice theory and fan diagrams in the low-energy Dirac theory. It is shown that the spin-Chern number can takes an arbitrary high value for certain QH systems. This is a new type of topological insulators, which we may call high spin-Chern insulators. Samples may be provided by graphene on the SiC substrate with ferromagnetic order, transition-metal dichalcogenides with ferromagnetic order, transition-metal oxide with antiferromagnetic order and silicene with ferromagnetic order. Actually high spin-Chern insulators are ubiquitous in any systems with magnetic order. Nevertheless, the honeycomb system would provide us with unique materials for practical materialization. PMID:24310394

  20. High Spin-Chern Insulators with Magnetic Order

    NASA Astrophysics Data System (ADS)

    Ezawa, Motohiko

    2013-12-01

    As a topological insulator, the quantum Hall (QH) effect is indexed by the Chern and spin-Chern numbers and . We have only in conventional QH systems. We investigate QH effects in generic monolayer honeycomb systems. We search for spin-resolved characteristic patterns by exploring Hofstadter's butterfly diagrams in the lattice theory and fan diagrams in the low-energy Dirac theory. It is shown that the spin-Chern number can takes an arbitrary high value for certain QH systems. This is a new type of topological insulators, which we may call high spin-Chern insulators. Samples may be provided by graphene on the SiC substrate with ferromagnetic order, transition-metal dichalcogenides with ferromagnetic order, transition-metal oxide with antiferromagnetic order and silicene with ferromagnetic order. Actually high spin-Chern insulators are ubiquitous in any systems with magnetic order. Nevertheless, the honeycomb system would provide us with unique materials for practical materialization.

  1. Spin constraints on nuclear energy density functionals

    NASA Astrophysics Data System (ADS)

    Robledo, L. M.; Bernard, R. N.; Bertsch, G. F.

    2014-02-01

    The Gallagher-Moszkowski rule in the spectroscopy of odd-odd nuclei imposes a new spin constraint on the energy functionals for self-consistent mean field theory. The commonly used parametrization of the effective three-body interaction in the Gogny and Skyrme families of energy functionals is ill suited to satisfy the spin constraint. In particular, the Gogny parametrization of the three-body interaction has the spin dependence opposite to that required by the observed spectra. The two-body part has a correct sign, but in combination the rule is violated as often as not. We conclude that a new functional form is needed for the effective three-body interaction that can take into better account the different spin-isospin channels of the interaction.

  2. Consistent interactions for high-spin fermion fields

    NASA Astrophysics Data System (ADS)

    Vrancx, Tom; de Cruz, Lesley; Ryckebusch, Jan; Vancraeyveld, Pieter

    2011-10-01

    We address the issue of consistent interactions for off-shell fermion fields of arbitrary spin. These interactions play a crucial role in the quantum hadrodynamical description of high-spin baryon resonances in hadronic processes. The Rarita-Schwinger (R-S) description of high-spin fermion fields involves unphysical degrees of freedom associated with their lower-spin content. These enter the interaction if not eliminated outright. The invariance condition of the interaction under the unconstrained R-S gauge removes the lower-spin content of the fermion propagator and leads to a consistent description of the interaction. We develop the most general consistent interaction structure for high-spin fermions. We find that the power of the momentum dependence of a consistent interaction rises with the spin of the fermion field. This leads to unphysical structures in the energy dependence of the computed tree-level cross sections when the short-distance physics is cut off with standard hadronic form factors. A spin-dependent hadronic form factor is proposed that suppresses the unphysical artifacts.

  3. Direct measurements of spin propagation in organic spin valves by low-energy muon spin rotation

    NASA Astrophysics Data System (ADS)

    Drew, Alan

    2013-03-01

    Organic semiconductors fall into a class of materials that shows significant potential for future applications, but many of the fundamental mechanisms of spin relaxation and transport are not understood. As a result, the field is becoming extremely topical, but there is a need for suitable techniques that can yield information on intrinsic spin dynamics and transport in organic materials. I will present Low Energy Muon Spin Rotation measurements and demonstrate that this technique can directly measure the depth resolved spin polarisation of charge carriers in organic spin injection devices. I will then go on to show that it is possible to separate out the various contributions to spin decoherence, differentiating between interface and bulk effects. By correlating macroscopic measurements with these separated interfacial and bulk effects, I will present evidence that it is possible to engineer interfaces in organic spintronic devices. Finally, I will present some of the latest results on how spin injection and transport depend on bias voltage. Research funded by the EU 7th Framework NMP Program (``HINTS'' NMP3-SL-2011-263104) and the European Research Council (``MuSES'' 307593).

  4. High-spin rotational bands in 123I

    NASA Astrophysics Data System (ADS)

    Singh, Purnima; Singh, A. K.; Wilson, A. N.; Ragnarsson, I.; Hübel, H.; Bürger, A.; Carpenter, M. P.; Chmel, S.; Fallon, P.; Hagemann, G. B.; Herskind, B.; Ha, Hoa; Janssens, R. V. F.; Juhász, K.; Kardan, A.; Khoo, T. L.; Kondev, G.; Korichi, A.; Lauritsen, T.; Nyakó, B. M.; Rogers, J.; Sletten, G.; Timár, J.; Zhu, S.

    2012-12-01

    High-spin states in 123I were populated in the reaction 80Se(48Ca,p4n)123I at a beam energy of 207 MeV and γ-ray coincidence events were measured using the Gammasphere spectrometer. Three weakly populated, high-spin rotational bands have been discovered with characteristics similar to those of the long collective bands recently observed in other nuclei of this mass region. Configuration assignments are proposed based on calculations within the framework of the cranked Nilsson-Strutinsky approach.

  5. Properties of the low-spin high-spin interface during the relaxation of spin-crossover materials, investigated through an electro-elastic model

    SciTech Connect

    Slimani, A.; Boukheddaden, K. Varret, F.; Nishino, M.; CREST, JST, 4-1-8 Honcho Kawaguchi, Saitama 332-0012 ; Miyashita, S.; Department of Physics, Graduate School of Science, The University of Tokyo, Bunkyo-Ku, Tokyo

    2013-11-21

    The present work is devoted to the spatio-temporal investigations of spin-crossover lattices during their thermal relaxation from high- to low-spin state. The analysis is performed using Monte Carlo simulations on a distortable 2D lattice the sites of which are occupied by high-spin (HS) or low-spin (LS) atoms. The lattice is circular in shape and the HS to LS transformation results in single domain nucleation followed by growth and propagation processes. The evolution of the LS:HS interface is monitored during the relaxation process, through the mapping of spin states, displacement fields, local stresses, and elastic energy. The results show a curved interface, the curvature of which is reversed at the mid-transformation. The local stresses and elastic energy peak at the vicinity of the HS:LS interface, with sizeable dependence upon the position along the front line which evidences the edge effects.

  6. Triaxiality and exotic rotations at high spins in 134Ce

    NASA Astrophysics Data System (ADS)

    Petrache, C. M.; Guo, S.; Ayangeakaa, A. D.; Garg, U.; Matta, J. T.; Nayak, B. K.; Patel, D.; Carpenter, M. P.; Chiara, C. J.; Janssens, R. V. F.; Kondev, F. G.; Lauritsen, T.; Seweryniak, D.; Zhu, S.; Ghugre, S. S.; Palit, R.

    2016-06-01

    High-spin states in 134Ce have been investigated using the 116Cd(22Ne,4 n ) reaction and the Gammasphere array. The level scheme has been extended to an excitation energy of ˜30 MeV and spin ˜54 ℏ . Two new dipole bands and four new sequences of quadrupole transitions were identified. Several new transitions have been added to a number of known bands. One of the strongly populated dipole bands was revised and placed differently in the level scheme, resolving a discrepancy between experiment and model calculations reported previously. Configurations are assigned to the observed bands based on cranked Nilsson-Strutinsky calculations. A coherent understanding of the various excitations, both at low and high spins, is thus obtained, supporting an interpretation in terms of coexistence of stable triaxial, highly deformed, and superdeformed shapes up to very high spins. Rotations around different axes of the triaxial nucleus, and sudden changes of the rotation axis in specific configurations, are identified, further elucidating the nature of high-spin collective excitations in the A =130 mass region.

  7. High-Spin Structure of 102Ru

    NASA Astrophysics Data System (ADS)

    Sohler, D.; Timár, J.; Rainovski, G.; Joshi, P.; Starosta, K.; Fossan, D. B.; Molnár, J.; Wadsworth, R.; Algora, A.; Bednarczyk, P.; Curien, D.; Dombrádi, Zs.; Duchene, G.; Gizon, A.; Gizon, J.; Jenkins, D. G.; Koike, T.; Krasznahorkay, A.; Paul, E. S.; Raddon, P. M.; Scheurer, J. N.; Simons, A. J.; Vaman, C.; Wilkinson, A. R.; Zolnai, L.

    2005-11-01

    High-spin states in the nucleus 102Ru have been studied through the 96Zr(13C,α3n) reaction using the EUROBALL IV γ-ray spectrometer accompanied by the DIAMANT array for the detection of charged particles. All previously known bands have been extended to higher spins and additional bands have been found. Comparing the experimental Routhians and aligned angular momenta to the predictions of Woods-Saxon TRS calculations, vh11/2(d5/2,g7/2) configurations have been assigned to the observed negative-parity bands.

  8. High-Spin Structure of 102Ru

    SciTech Connect

    Sohler, D.; Timar, J.; Molnar, J.; Algora, A.; Dombradi, Zs.; Krasznahorkay, A.; Zolnai, L.; Rainovski, G.; Joshi, P.; Wadsworth, R.; Jenkins, D.G.; Raddon, P.M.; Simons, A.J.; Wilkinson, A.R.; Starosta, K.; Fossan, D.B.; Bednarczyk, P.; Curien, D.; Duchene, G.; Gizon, A.

    2005-11-21

    High-spin states in the nucleus 102Ru have been studied through the 96Zr(13C,{alpha}3n) reaction using the EUROBALL IV {gamma}-ray spectrometer accompanied by the DIAMANT array for the detection of charged particles. All previously known bands have been extended to higher spins and additional bands have been found. Comparing the experimental Routhians and aligned angular momenta to the predictions of Woods-Saxon TRS calculations, vh11/2(d5/2,g7/2) configurations have been assigned to the observed negative-parity bands.

  9. Spin transport in intermediate-energy heavy-ion collisions as a probe of in-medium spin-orbit interactions

    NASA Astrophysics Data System (ADS)

    Xia, Yin; Xu, Jun; Li, Bao-An; Shen, Wen-Qing

    2016-11-01

    The spin up-down splitting of collective flows in intermediate-energy heavy-ion collisions as a result of the nuclear spin-orbit interaction is investigated within a spin- and isospin-dependent Boltzmann-Uehling-Uhlenbeck transport model SIBUU12. Using a Skyrme-type spin-orbit coupling quadratic in momentum, we found that the spin splittings of the directed flow and elliptic flow are largest in peripheral Au+Au collisions at beam energies of about 100-200 MeV/nucleon, and the effect is considerable even in smaller systems especially for nucleons with high transverse momenta. The collective flows of light clusters of different spin states are also investigated using an improved dynamical coalescence model with spin. Our study can be important in understanding the properties of in-medium nuclear spin-orbit interactions once the spin-dependent observables proposed in this work can be measured.

  10. Spin-bag mechanism of high-temperature superconductivity

    NASA Technical Reports Server (NTRS)

    Schrieffer, J. R.; Wen, X.-G.; Zhang, S.-C.

    1988-01-01

    A new approach to the theory of high-temperature superconductivity is proposed, based on the two-dimensional antiferromagnetic spin correlations observed in these materials over distances large compared to the lattice spacing. The spin ordering produces an electronic pseudogap which is locally suppressed by the addition of a hole. This suppression forms a bag inside which the hole is self-consistently trapped. Two holes are attracted by sharing a common bag. The resulting pairing interaction leads to a superconducting energy gap which is nodeless over the Femri surface.

  11. Gross shell structure at high spin in heavy nuclei

    SciTech Connect

    Deleplanque, Marie-Agnes; Frauendorf, Stefan; Pashkevich, Vitaly V.; Chu, S.Y.; Unzhakova, Anja

    2003-10-07

    Experimental nuclear moments of inertia at high spins along the yrast line have been determined systematically and found to differ from the rigid-body values. The difference is attributed to shell effect and these have been calculated microscopically. The data and quantal calculations are interpreted by means of the semiclassical Periodic Orbit Theory. From this new perspective, features in the moments of inertia as a function of neutron number and spin, as well as their relation to the shell energies can be understood. Gross shell effects persist up to the highest angular momenta observed.

  12. Nuclear states and shapes at high spin. [Good review

    SciTech Connect

    Diamond, R.M.

    1980-08-01

    As angular momentum is added to a nucleus, the balance of forces acting upon it to determine its shape, moment of inertia, mode of rotation, and type of level structure may undergo a series of changes. At relatively low spins a deformed nucleus will rotate collectively, and one may see the effect of Coriolis antipairing in gradually increasing the moment of inertia. Around spin 12 to 16 h-bar there may be an abrupt change (backbending) when a pair of high-j nucleons unpairs and the nucleons align with the axis of rotation; this process allows the nucleus to slow its collective rotation. This process, the start of a sharing of angular momentum between single-particle motion and the collective rotation, gives a lower total energy and corresponds to a change toward triaxiality in the shape of the nucleus. At much higher spins discrete ..gamma..-ray transitions can no longer be observed. This is the regime of continuum spectra; all the information on these high-spin states (to 65 h-bar) is contained in these continuum cascades. Knowledge is accumulating on how to study these spectra, experimentally and theoretically, and new techniques offer promise of revealing a great deal of information about the shapes and properties of very high spin states. 71 references, 34 figures.

  13. [Spin dependent phenomena in medium energy physics]. Technical progress report

    SciTech Connect

    Souder, P.A.

    1992-11-01

    The Syracuse University Medium Energy Physics Group was actively engaged in several research projects. A laser was used to polarize muonic atoms with the goal of measuring fundamental spin-dependent parameters in the reaction {mu}{sup {minus}} + {sup 3}He {yields} {sup 3}H + {nu}. Time-averaged polarizations of 26.8{plus_minus}2.3% were achieved for the muon in muonic {sup 3}He. The new approach uses atomic spin-dependent reactions between laser polarized Rb vapor and muonic helium. To exploit these high polarizations in a muon capture experiment an ion chamber which will detect the recoil tritons and also serve as a polarizing cell. Final data-taking will begin for an experiment to measure the spin-dependent structure functions of the neutron. A 288-element hodoscope system which features good timing and precise mechanical tolerances was constructed and evaluated.

  14. High-spin molecular resonances in 12C + 12C

    NASA Astrophysics Data System (ADS)

    Uegaki, E.; Abe, Y.

    2016-05-01

    Resonances observed in the 12C + 12C collisions are studied with a molecular model. At high spins J = 10-18, a stable dinuclear configuration is found to be an equator-equator touching one. Firstly, normal modes have been solved around the equilibrium, with spin J and K-quantum number being specified for rotation of the whole system. Secondly, with respect to large centrifugal energy, Coriolis coupling has been diagonalized among low-lying 11 states of normal-mode excitations, which brings K-mixing. The analyses of decay widths and excitation functions have been done. The molecular ground state exhibits alignments of the orbital angular momentum and the 12C spins, while some of the molecular excited states exhibit disalignments with small widths. Those results are surprisingly in good agreement with the experiments, which will light up a new physical picture of the highspin 12C + 12C resonances.

  15. High-spin spectroscopy of 140Nd

    NASA Astrophysics Data System (ADS)

    Leguillon, R.; Petrache, C. M.; Zerrouki, T.; Konstantinopoulos, T.; Hauschild, K.; Korichi, A.; Lopez-Martens, A.; Frauendorf, S.; Ragnarsson, I.; Greenlees, P. T.; Jakobsson, U.; Jones, P.; Julin, R.; Juutinen, S.; Ketelhut, S.; Leino, M.; Nieminen, P.; Nyman, M.; Peura, P.; Rahkila, P.; Ruotsalainen, P.; Sandzelius, M.; Saren, J.; Scholey, C.; Sorri, J.; Uusitalo, J.; Hübel, H.; Neußer-Neffgen, A.; Al-Khatib, A.; Bürger, A.; Nenoff, N.; Singh, A. K.; Curien, D.; Hagemann, G. B.; Herskind, B.; Sletten, G.; Fallon, P.; Görgen, A.; Bednarczyk, P.; Cullen, D. M.

    2013-07-01

    The population of the high-spin states in 140Nd was investigated using the reaction 96Zr(48Ca,4n). The results from two experiments, one with the EUROBALL array and one with the JUROGAM II+RITU+GREAT setup employing the recoil decay tagging technique, have been combined to develop a very detailed level scheme for 140Nd. Twelve bands of quadrupole transitions and eleven bands of dipole transitions were identified and their connections to low-lying states were established. Calculations using the cranked Nilsson-Strutinsky and the tilted axis cranking models were used to interpret the observed structures. The overall good agreement between the experimental results and the calculations assuming a triaxial shape of the nucleus strongly support the existence of a stable triaxial shape at high spins in this mass region.

  16. Spin drift in highly doped n-type Si

    SciTech Connect

    Kameno, Makoto; Ando, Yuichiro; Shinjo, Teruya; Koike, Hayato; Sasaki, Tomoyuki; Oikawa, Tohru; Suzuki, Toshio; Shiraishi, Masashi

    2014-03-03

    A quantitative estimation of spin drift velocity in highly doped n-type silicon (Si) at 8 K is presented in this letter. A local two-terminal Hanle measurement enables the detection of a modulation of spin signals from the Si as a function of an external electric field, and this modulation is analyzed by using a spin drift-diffusion equation and an analytical solution of the Hanle-type spin precession. The analyses reveal that the spin drift velocity is linearly proportional to the electric field. The contribution of the spin drift effect to the spin signals is crosschecked by introducing a modified nonlocal four-terminal method.

  17. High-spin and low-spin mixed state in LaSrCoO4 : An ab initio study

    NASA Astrophysics Data System (ADS)

    Wu, Hua

    2010-03-01

    Spin state is an important issue for many cobaltates, and an intermediate spin (IS) state having a half-filled eg orbital may well be expected for a Co3+ ion in a CoO6 octahedron with a remarkable tetragonal distortion. Here the single-layered perovskite cobaltate LaSrCoO4 , which has a notable tetragonal elongation, is investigated for its spin state and electronic structure, through a set of local-spin-density approximation plus Hubbard U (LSDA+U) calculations including also the multiplet effect and spin-orbit coupling. Counterintuitively, our calculations evidence that the IS state is not the ground state and it would, even if being so, give rise to a wrong ferromagnetic half-metallic solution. We find that a strong band hybridization significantly suppresses a multiplet energy splitting of the IS state. Instead, a high-spin (HS) and low-spin (LS) mixed state turns out to have the lowest total energy among all possibly combined spin states. Moreover, the mixed HS+LS ground state well accounts for the experimental paramagnetic insulating behavior, the effective magnetic moment, and the observed optical spectral features. We also predict that LaSrCoO4 in the mixed HS+LS ground state has a sizeable out-of-plane orbital moment and a local lattice distortion, which would motivate experimental studies.

  18. Unexpected suppression of spin-lattice relaxation via high magnetic field in a high-spin iron(iii) complex.

    PubMed

    Zadrozny, Joseph M; Graham, Michael J; Krzyaniak, Matthew D; Wasielewski, Michael R; Freedman, Danna E

    2016-08-01

    A counterintuitive three-order of magnitude slowing of the spin-lattice relaxation rate is observed in a high spin qubit at high magnetic field via multifrequency pulsed electron paramagnetic resonance measurements. PMID:27463410

  19. Spin Hall magnetoresistance at high temperatures

    SciTech Connect

    Uchida, Ken-ichi; Qiu, Zhiyong; Kikkawa, Takashi; Iguchi, Ryo; Saitoh, Eiji

    2015-02-02

    The temperature dependence of spin Hall magnetoresistance (SMR) in Pt/Y{sub 3}Fe{sub 5}O{sub 12} (YIG) bilayer films has been investigated in a high temperature range from room temperature to near the Curie temperature of YIG. The experimental results show that the magnitude of the magnetoresistance ratio induced by the SMR monotonically decreases with increasing the temperature and almost disappears near the Curie temperature. We found that, near the Curie temperature, the temperature dependence of the SMR in the Pt/YIG film is steeper than that of a magnetization curve of the YIG; the critical exponent of the magnetoresistance ratio is estimated to be 0.9. This critical behavior of the SMR is attributed mainly to the temperature dependence of the spin-mixing conductance at the Pt/YIG interface.

  20. The spin bag mechanism of high temperature superconductivity

    NASA Technical Reports Server (NTRS)

    Schrieffer, J. R.; Wen, X.-G.; Zhang, S.-C.

    1989-01-01

    In oxide superconductors the local suppression of antiferromagnetic correlations in the vicinity of a hole lowers the energy of the system. This quasi two-dimensional bag of weakened spin order follows the hole in its motion. In addition, holes prefer to share a bag, leading to a strong pairing attraction and a high Tc superconductivity. There are many experimental consequences of this mechanism for both the superconducting and normal phases.

  1. Nuclear moments of inertia at high spin

    SciTech Connect

    Deleplanque, M.A.

    1982-10-01

    The competition between collective motion and alignment at high spin can be evaluated by measuring two complementary dynamic moments of inertia. The first, I band, measured in ..gamma..-..gamma.. correlation experiments, relates to the collective properties of the nucleus. A new moment of inertia I/sub eff/ is defined here, which contains both collective and alignment effects. Both of these can be measured in continuum ..gamma..-ray spectra of rotational nuclei up to high frequencies. The evolution of ..gamma..-ray spectra for Er nuclei from mass 160 to 154 shows that shell effects can directly be observed in the spectra of the lighter nuclei.

  2. Low-Energy Spin Dynamics of the Honeycomb Spin Liquid Beyond the Kitaev Limit

    NASA Astrophysics Data System (ADS)

    Song, Xue-Yang; You, Yi-Zhuang; Balents, Leon

    2016-07-01

    We investigate the generic features of the low energy dynamical spin structure factor of the Kitaev honeycomb quantum spin liquid perturbed away from its exact soluble limit by generic symmetry-allowed exchange couplings. We find that the spin gap persists in the Kitaev-Heisenberg model, but generally vanishes provided more generic symmetry-allowed interactions exist. We formulate the generic expansion of the spin operator in terms of fractionalized Majorana fermion operators according to the symmetry enriched topological order of the Kitaev spin liquid, described by its projective symmetry group. The dynamical spin structure factor displays power-law scaling bounded by Dirac cones in the vicinity of the Γ , K , and K' points of the Brillouin zone, rather than the spin gap found for the exactly soluble point.

  3. Doping dependence of spin excitations and its correlations with high-temperature superconductivity in iron pnictides

    PubMed Central

    Wang, Meng; Zhang, Chenglin; Lu, Xingye; Tan, Guotai; Luo, Huiqian; Song, Yu; Wang, Miaoyin; Zhang, Xiaotian; Goremychkin, E.A.; Perring, T.G.; Maier, T.A.; Yin, Zhiping; Haule, Kristjan; Kotliar, Gabriel; Dai, Pengcheng

    2013-01-01

    High-temperature superconductivity in iron pnictides occurs when electrons and holes are doped into their antiferromagnetic parent compounds. Since spin excitations may be responsible for electron pairing and superconductivity, it is important to determine their electron/hole-doping evolution and connection with superconductivity. Here we use inelastic neutron scattering to show that while electron doping to the antiferromagnetic BaFe2As2 parent compound modifies the low-energy spin excitations and their correlation with superconductivity (<50 meV) without affecting the high-energy spin excitations (>100 meV), hole-doping suppresses the high-energy spin excitations and shifts the magnetic spectral weight to low-energies. In addition, our absolute spin susceptibility measurements for the optimally hole-doped iron pnictide reveal that the change in magnetic exchange energy below and above Tc can account for the superconducting condensation energy. These results suggest that high-Tc superconductivity in iron pnictides is associated with both the presence of high-energy spin excitations and a coupling between low-energy spin excitations and itinerant electrons. PMID:24301219

  4. Low energy spin excitations in chromium metal

    SciTech Connect

    Pynn, R.; Azuah, R.T.; Stirling, W.G.; Kulda, J.

    1997-12-31

    Neutron scattering experiments with full polarization analysis have been performed with a single crystal of chromium to study the low-energy spin fluctuations in the transverse spin density wave (TSDW) state. A number of remarkable results have been found. Inelastic scattering observed close to the TSDW satellite positions at (1 {+-} {delta},0,0) does not behave as expected for magnon scattering. In particular, the scattering corresponds to almost equally strong magnetization fluctuations both parallel and perpendicular to the ordered moments of the TSDW phase. As the Neel temperature is approached from below, scattering at the commensurate wavevector (1,0,0) increases in intensity as a result of critical scattering at silent satellites (1,0, {+-} {delta}) being included within the spectrometer resolution function. This effect, first observed by Sternlieb et al, does not account for all of the inelastic scattering around the (1,0,0) position, however, Rather, there are further collective excitations, apparently emanating from the TSDW satellites, which correspond to magnetic fluctuations parallel to the ordered TSDW moments. These branches have a group velocity that is close to that of (1,0,0) longitudinal acoustic (LA) phonons, but assigning their origin to magneto-elastic scattering raises other unanswered questions.

  5. High spin-filter efficiency and Seebeck effect through spin-crossover iron-benzene complex.

    PubMed

    Yan, Qiang; Zhou, Liping; Cheng, Jue-Fei; Wen, Zhongqian; Han, Qin; Wang, Xue-Feng

    2016-04-21

    Electronic structures and coherent quantum transport properties are explored for spin-crossover molecule iron-benzene Fe(Bz)2 using density functional theory combined with non-equilibrium Green's function. High- and low-spin states are investigated for two different lead-molecule junctions. It is found that the asymmetrical T-shaped contact junction in the high-spin state behaves as an efficient spin filter while it has a smaller conductivity than that in the low-spin state. Large spin Seebeck effect is also observed in asymmetrical T-shaped junction. Spin-polarized properties are absent in the symmetrical H-shaped junction. These findings strongly suggest that both the electronic and contact configurations play significant roles in molecular devices and metal-benzene complexes are promising materials for spintronics and thermo-spintronics. PMID:27389217

  6. High spin-filter efficiency and Seebeck effect through spin-crossover iron-benzene complex

    NASA Astrophysics Data System (ADS)

    Yan, Qiang; Zhou, Liping; Cheng, Jue-Fei; Wen, Zhongqian; Han, Qin; Wang, Xue-Feng

    2016-04-01

    Electronic structures and coherent quantum transport properties are explored for spin-crossover molecule iron-benzene Fe(Bz)2 using density functional theory combined with non-equilibrium Green's function. High- and low-spin states are investigated for two different lead-molecule junctions. It is found that the asymmetrical T-shaped contact junction in the high-spin state behaves as an efficient spin filter while it has a smaller conductivity than that in the low-spin state. Large spin Seebeck effect is also observed in asymmetrical T-shaped junction. Spin-polarized properties are absent in the symmetrical H-shaped junction. These findings strongly suggest that both the electronic and contact configurations play significant roles in molecular devices and metal-benzene complexes are promising materials for spintronics and thermo-spintronics.

  7. Spin-polaron theory of high-{Tc} superconductivity: I, spin polarons and high-{Tc} pairing

    SciTech Connect

    Wood, R.F.

    1993-06-01

    The concept of a spin polaron is introduced and contrasted with the more familiar ionic polaron picture. A brief review of aspects of ionic bipolaronic superconductivity is given with particular emphasis on the real-space pairing and true Bose condensation characteristics. The formation energy of spin polarons is then calculated in analogy with ionic polarons. The spin-flip energy of a Cu spin in an antiferromagnetically aligned CuO{sub 2} plane is discussed. It is shown that the introduction of holes into the CuO{sub 2} planes will always lead to the destruction of long-range AF ordering due to the formation of spin polarons. The pairing of two spin polarons can be expected because of the reestablishment of local (short-range) AF ordering; the magnitude of the pairing energy is estimated using a simplified model. The paper closes with a brief discussion of the formal theory of spin polarons.

  8. High spin polarization and spin splitting in equiatomic quaternary CoFeCrAl Heusler alloy

    NASA Astrophysics Data System (ADS)

    Bainsla, Lakhan; Mallick, A. I.; Coelho, A. A.; Nigam, A. K.; Varaprasad, B. S. D. Ch. S.; Takahashi, Y. K.; Alam, Aftab; Suresh, K. G.; Hono, K.

    2015-11-01

    In this paper, we investigate CoFeCrAl alloy by means of ab-initio electronic structure calculations and various experimental techniques. The alloy is found to exist in the B2-type cubic Heusler structure, which is very similar to Y-type (or LiMgPdSn prototype) structure with space group F-43m (#216). Saturation magnetization (MS) of about 2 μB/f.u. is observed at 8 K under ambient pressure, which is in good agreement with the Slater-Pauling rule. MS values are found to be independent of pressure, which is a prerequisite for half-metals. The ab-initio electronic structure calculations predict half-metallicity for the alloy with a spin slitting energy of 0.31 eV. Importantly, this system shows a high current spin polarization value of 0.67±0.02, as deduced from the point contact Andreev reflection measurements. Linear dependence of electrical resistivity with temperature indicates the possibility of reasonably high spin polarization at elevated temperatures (~150 K) as well. All these suggest that CoFeCrAl is a promising material for the spintronic devices.

  9. Development of a spin polarized low energy electron diffraction system.

    PubMed

    Pradeep, A V; Roy, Arnab; Kumar, P S Anil; Kirschner, J

    2016-02-01

    We have designed and constructed a spin polarized low energy electron diffraction system working in the reflected electron pulse counting mode. This system is capable of measuring asymmetries due to spin-orbit and exchange interactions. Photoemission from a strained GaAs/GaAsP super lattice is used as the source of spin polarized electrons. Spin-orbit asymmetry is evaluated for Ir(100) single crystal at various energies. Subsequently, exchange asymmetry has been evaluated on 40 monolayer Fe deposited on Ir(100). This instrument proves to be useful in understanding structure and magnetism at surfaces. PMID:26931865

  10. Development of a spin polarized low energy electron diffraction system

    NASA Astrophysics Data System (ADS)

    Pradeep, A. V.; Roy, Arnab; Kumar, P. S. Anil; Kirschner, J.

    2016-02-01

    We have designed and constructed a spin polarized low energy electron diffraction system working in the reflected electron pulse counting mode. This system is capable of measuring asymmetries due to spin-orbit and exchange interactions. Photoemission from a strained GaAs/GaAsP super lattice is used as the source of spin polarized electrons. Spin-orbit asymmetry is evaluated for Ir(100) single crystal at various energies. Subsequently, exchange asymmetry has been evaluated on 40 monolayer Fe deposited on Ir(100). This instrument proves to be useful in understanding structure and magnetism at surfaces.

  11. High-spin structure of {sup 102}Ru

    SciTech Connect

    Sohler, D.; Timar, J.; Molnar, J.; Dombradi, Zs.; Krasznahorkay, A.; Zolnai, L.; Rainovski, G.; Joshi, P.; Wadsworth, R.; Jenkins, D.G.; Raddon, P.M.; Simons, A.J.; Wilkinson, A.R.; Starosta, K.; Fossan, D.B.; Koike, T.; Vaman, C.; Algora, A.; Bednarczyk, P.; Curien, D.

    2005-06-01

    High-spin states in the nucleus {sup 102}Ru have been investigated via the {sup 96}Zr({sup 13}C,{alpha}3n) reaction at beam energies of 51 and 58 MeV, using the euroball IV {gamma}-ray spectrometer and the diamant charged particle array. Several new high-spin bands have been established. The ground-state band has been extended up to E{sub x}{approx}12 MeV with I{sup {pi}}=(26{sup +}); the previously published negative-parity bands have been extended up to E{sub x}{approx}11 and {approx} 9 MeV with I{sup {pi}}=(23{sup -}) and (20{sup -}), respectively. The deduced high-spin structure has been compared with Woods-Saxon total Routhian surface calculations and, on the basis of the measured Routhians, aligned angular momenta, and B(M1)/B(E2) ratios, {nu}h{sub 11/2}(g{sub 7/2},d{sub 5/2}) configurations are suggested for the negative-parity structures.

  12. Band structures extending to very high spin in Xe126

    NASA Astrophysics Data System (ADS)

    Rønn Hansen, C.; Sletten, G.; Hagemann, G. B.; Herskind, B.; Jensen, D. R.; Bringel, P.; Engelhardt, C.; Hübel, H.; Neußer-Neffgen, A.; Singh, A. K.; Carpenter, M. P.; Janssens, R. V. F.; Khoo, T. L.; Lauritsen, T.; Bednarczyk, P.; Byrski, T.; Curien, D.; Benzoni, G.; Bracco, A.; Camera, F.; Leoni, S.; Clark, R. M.; Fallon, P.; Korichi, A.; Roccaz, J.; Maj, A.; Wilson, J. N.; Lisle, J. C.; Steinhardt, T.; Thelen, O.; Ødegård, S. W.

    2007-09-01

    High-spin states in Xe126 have been populated in the Se82(Ca48,4n)Xe126 reaction in two experiments, one at the VIVITRON accelerator in Strasbourg using the Euroball detector array, and a subsequent one with ATLAS at Argonne using the Gammasphere Ge-detector array. Levels and assignments made previously for Xe126 up to I=20 have been confirmed and extended. Four regular bands extending to a spin of almost I=60, which are interpreted as two pairs of signature partners with opposite parity, are identified for the first time. The α = 0 partner of each pair is connected to the lower-lying levels, whereas the two α = 1 partners remain floating. A fractional Doppler shift analysis of transitions in the strongest populated (π,α)=(-,0) band provides a value of 5.20.50.4 b for the transition quadrupole moment, which can be related to a minimum in the potential-energy surface calculated by the ULTIMATE CRANKER cranked shell-model code at ɛ≈0.35 and γ≈5°. The four lowest bands calculated for this minimum compare well with the two signature pairs experimentally observed over a wide spin range. A sharp upbend at ℏω~1170 keV is interpreted as a crossing with a band involving the j15/2 neutron orbital, for which pairing correlations are expected to be totally quenched. The four long bands extend to within ˜5 spin units of a crossing with an yrast line defined by calculated hyperdeformed transitions and will serve as important stepping stones into the spin region beyond 60ħ for future experiments.

  13. Evidence for High Spin States in 70Ga

    NASA Astrophysics Data System (ADS)

    Tan, C. L.; Haring-Kaye, R. A.; Jones, K. D.; Le, K. Q.; Döring, J.; Abromeit, B.; Dungan, R.; Lubna, R.; Tabor, S. L.; Tai, P.-L.; Tripathi, V.; Vonmoss, J. M.; Morrow, S. I.

    2015-10-01

    High-spin states in the odd-odd 70Ga nucleus were populated at Florida State University using the 62Ni(14C, αpn) fusion-evaporation reaction at a beam energy of 50 MeV. Gamma rays that depopulated the 70Ga excited states were recorded in coincidence with a Compton-suppressed Ge array consisting of three clover detectors and seven single-crystal detectors. The existing 70Ga level scheme was modified, enhanced, and extended to higher spin with the addition of eight new transitions based on the analysis of double- and triple-coincidence γ-ray spectra. Five of these transitions are associated with a new rotational band that may be based on the occupation of the g9 / 2 orbital by the unpaired proton and neutron. The normalized energy differences between adjacent spin states in this new band indicate a signature-splitting pattern that is characteristic of other such bands in neighboring odd-odd nuclei. Similarly, the kinematic moments of inertia deduced for this decay sequence evolve with angular frequency in a manner typical of analogous bands in other odd-odd nuclei in this mass region.

  14. High-spin structures in the 129Xe nucleus

    NASA Astrophysics Data System (ADS)

    Huang, Y.; Xiao, Z. G.; Zhu, S. J.; Qi, C.; Xu, Q.; Cheng, W. J.; Li, H. J.; Lyu, L. M.; Wang, R. S.; Yan, W. H.; Yi, H.; Zhang, Y.; Chen, Q. M.; He, C. Y.; Hu, S. P.; Li, C. B.; Li, H. W.; Luo, P. W.; Wu, X. G.; Wu, Y. H.; Zheng, Y.; Zhong, J.

    2016-06-01

    High-spin states in the 129Xe nucleus are studied with the reaction 124Sn(9Be,4 n ) at a beam energy of 36 MeV. The level scheme is extended significantly. For the positive-parity band, the α =+1 /2 and the α =-1 /2 signature components are combined to form a complete band structure based on the 3 /2+ state with spin and parity up to 21 /2+ . For the negative-parity band based on the 11 /2- state, the α =+1 /2 signature component is newly established and both the α =+1 /2 and the α =-1 /2 signature components also form a complete band structure up to the 35 /2- state. The positive- and negative-parity bands are proposed to originate from ν d3 /23 /2+[402 ] and ν h11 /211 /2-[505 ] Nilsson configurations, respectively. A backbending is observed in the negative-parity band, which originates from the alignments of two h11 /2 protons according to crank shell model calculations. Based on the total Routhian surface and quasiparticle triaxial rotor model calculations, the negative-parity band is interpreted as a triaxially deformed shape with γ ≈-30∘ , while the positive-parity band is associated with γ softness, in accordance with previous studies. In the high-spin states, three decoupled bands and one oblate band with γ ≈-60∘ are newly identified. The systematics and other characteristics of these bands are discussed.

  15. Highly sensitive nanoscale spin-torque diode

    NASA Astrophysics Data System (ADS)

    Miwa, S.; Ishibashi, S.; Tomita, H.; Nozaki, T.; Tamura, E.; Ando, K.; Mizuochi, N.; Saruya, T.; Kubota, H.; Yakushiji, K.; Taniguchi, T.; Imamura, H.; Fukushima, A.; Yuasa, S.; Suzuki, Y.

    2014-01-01

    Highly sensitive microwave devices that are operational at room temperature are important for high-speed multiplex telecommunications. Quantum devices such as superconducting bolometers possess high performance but work only at low temperature. On the other hand, semiconductor devices, although enabling high-speed operation at room temperature, have poor signal-to-noise ratios. In this regard, the demonstration of a diode based on spin-torque-induced ferromagnetic resonance between nanomagnets represented a promising development, even though the rectification output was too small for applications (1.4 mV mW-1). Here we show that by applying d.c. bias currents to nanomagnets while precisely controlling their magnetization-potential profiles, a much greater radiofrequency detection sensitivity of 12,000 mV mW-1 is achievable at room temperature, exceeding that of semiconductor diode detectors (3,800 mV mW-1). Theoretical analysis reveals essential roles for nonlinear ferromagnetic resonance, which enhances the signal-to-noise ratio even at room temperature as the size of the magnets decreases.

  16. Optically tunable spin-exchange energy at donor:acceptor interfaces in organic solar cells

    SciTech Connect

    Li, Mingxing; Wang, Hongfeng; He, Lei; Zang, Huidong; Xu, Hengxing; Hu, Bin

    2014-07-14

    Spin-exchange energy is a critical parameter in controlling spin-dependent optic, electronic, and magnetic properties in organic materials. This article reports optically tunable spin-exchange energy by studying the line-shape characteristics in magnetic field effect of photocurrent developed from intermolecular charge-transfer states based on donor:acceptor (P3HT:PCBM) system. Specifically, we divide magnetic field effect of photocurrent into hyperfine (at low field < 10 mT) and spin-exchange (at high field > 10 mT) regimes. We observe that increasing photoexcitation intensity can lead to a significant line-shape narrowing in magnetic field effect of photocurrent occurring at the spin-exchange regime. We analyze that the line-shape characteristics is essentially determined by the changing rate of magnetic field-dependent singlet/triplet ratio when a magnetic field perturbs the singlet-triplet transition through spin mixing. Based on our analysis, the line-shape narrowing results indicate that the spin-exchange energy at D:A interfaces can be optically changed by changing photoexcitation intensity through the interactions between intermolecular charge-transfer states. Therefore, our experimental results demonstrate an optical approach to change the spin-exchange energy through the interactions between intermolecular charge-transfer states at donor:acceptor interface in organic materials.

  17. Lifetimes Measurement for High Spin States in 107Ag

    NASA Astrophysics Data System (ADS)

    Yao, S. H.; Wu, X. G.; He, C. Y.; Zhang, B.; Zheng, Y.; Li, G. S.; Li, C. B.; Hu, S. P.; Cao, X. P.; Yu, B. B.; Zhu, L. H.; Xu, C.; Cheng, Y. Y.

    2013-11-01

    The excited states in 107Ag were populated through the heavy-ion fusion-evaporation reaction 100Mo (11B, 4n) 107Ag at a beam energy of 46 MeV. 12 Compton suppressed HPGe detectors and 2 planar HPGe detectors were employed to detect the de-excited γ rays from the reaction residues. Lifetimes of high spin states in 107Ag have been measured using the Doppler shift attenuation method (DSAM) and the deduced B(M1) and B(E2) transition probabilities have been derived from the measured lifetimes.

  18. Energy efficient hybrid computing systems using spin devices

    NASA Astrophysics Data System (ADS)

    Sharad, Mrigank

    Emerging spin-devices like magnetic tunnel junctions (MTJ's), spin-valves and domain wall magnets (DWM) have opened new avenues for spin-based logic design. This work explored potential computing applications which can exploit such devices for higher energy-efficiency and performance. The proposed applications involve hybrid design schemes, where charge-based devices supplement the spin-devices, to gain large benefits at the system level. As an example, lateral spin valves (LSV) involve switching of nanomagnets using spin-polarized current injection through a metallic channel such as Cu. Such spin-torque based devices possess several interesting properties that can be exploited for ultra-low power computation. Analog characteristic of spin current facilitate non-Boolean computation like majority evaluation that can be used to model a neuron. The magneto-metallic neurons can operate at ultra-low terminal voltage of ˜20mV, thereby resulting in small computation power. Moreover, since nano-magnets inherently act as memory elements, these devices can facilitate integration of logic and memory in interesting ways. The spin based neurons can be integrated with CMOS and other emerging devices leading to different classes of neuromorphic/non-Von-Neumann architectures. The spin-based designs involve `mixed-mode' processing and hence can provide very compact and ultra-low energy solutions for complex computation blocks, both digital as well as analog. Such low-power, hybrid designs can be suitable for various data processing applications like cognitive computing, associative memory, and currentmode on-chip global interconnects. Simulation results for these applications based on device-circuit co-simulation framework predict more than ˜100x improvement in computation energy as compared to state of the art CMOS design, for optimal spin-device parameters.

  19. Distinctive Reaction Pathways at Base Metals in High-Spin Organometallic Catalysts.

    PubMed

    Holland, Patrick L

    2015-06-16

    Inexpensive "base" metals are more affordable and sustainable than precious metals and also offer opportunities to discover new mechanisms for selective catalytic reactions. Base metal complexes can have high-spin electronic configurations that are rare in precious metal complexes. This Account describes some concepts relevant to high-spin organometallic complexes, focusing on our recent work with β-diketiminate complexes of iron and cobalt. Even though high-spin organometallic complexes have some unfamiliar spectroscopic properties, they can be studied using NMR spectroscopy as well as techniques that focus on the magnetism brought about by the unpaired electrons. Understanding the mechanisms of reactions using these complexes can be complicated, because complexes with a high-spin electronic configuration may need to change spin states to avoid high barriers for reaction. These spin-state changes can be rapid, and the ability of an excited spin state to "cut through" the barrier for a reaction can lead to spin acceleration. These concepts, originally developed by Poli, Shaik, Schwarz, and Harvey, are applied here to the fundamental organometallic reaction of β-hydride elimination (BHE). Experimentally validated density-functional calculations show spin acceleration in BHE using three-coordinate iron(II) and cobalt(II) complexes. A square-planar transition state is particularly beneficial for accelerating BHE when a high-spin iron(II) complex goes from an S = 2 ground state to an S = 1 transition state or when a high-spin cobalt(II) complex goes from an S = 3/2 ground state to an S = 1/2 transition state. The relative energies of the spin states can be controlled with the choice of the supporting ligand. Using an appropriate ligand, isomerization of 1-alkenes to their Z-2 isomers can be catalyzed in high yields using the cobalt(II) alkyl complexes as catalysts. Though an earlier paper attributed the regioselectivity and stereoselectivity to the preferred geometry

  20. High Spin Baryons in Quantum Mechanical Chromodynamics

    SciTech Connect

    Kirchbach, M.; Compean, C. B.

    2009-04-20

    A framework of quantum mechanical chromodynamics (QMCD) is developed with the aim to place the description of the nucleon on a comparable footing with Schroedinger's quantum mechanical treatment of the hydrogen atom. Such indeed turns out to be possible upon replacing the (e{sup -}-p) by a (q-qq) system, on the one hand, and the Coulomb potential by the recently reported by us exactly solvable trigonometric extension of the Cornell (TEC) potential, on the other. The TEC potential translates the inverse distance potential in ordinary flat space to a space of constant positive curvature, the 3D hypersphere, a reason for which both potentials have the SO(4) and SO(2, 1) symmetries in common. In effect, the nucleon spectrum, inclusive its {delta} branch, acquire the degeneracy patterns of the electron excitations with spin in {sup 1}H without copying them, however. There are two essential differences between the N({delta}) and H atom spectra. The first concerns the parity of the states which can be unnatural for the N and {delta} excitations due to compositeness of the diquark, the second refers to the level splittings in the baryon spectra which contain besides the Balmer term also its inverse of opposite sign. Our scheme reproduces the complete number of states (except the hybrid {delta}(1600)), predicts a total of 33 new resonances, and explains the splittings of the N and {delta} levels containing high-spin resonances. It also describes accurately the proton electric charge form factor. We here calculate the potential in momentum space (instantaneous effective gluon propagator) as a Fourier transform of the TEC potential and show that the concept of curvature allows to avoid the integral divergences suffered by schemes based on power potentials. We find a propagator that is finite at origin, likely to produce confinement. The advocated new potential picture allows for deconfinement too as effect of space flattening in the limit of infinite radius of the 3D

  1. Dipole-Dipole Interactions of High-spin Paramagnetic Centers in Disordered Systems

    SciTech Connect

    Maryasov, Alexander G.; Bowman, Michael K.; Tsvetkov, Yuri D.

    2007-09-13

    Dipole-dipole interactions between distant paramagnetic centers (PCs) where at least one PC has spin S>1/2 are examined. The results provide a basis for the application of pulsed DEER or PELDOR methods to the measurement of distances between PC involving high-spin species. A projection operator technique based on spectral decomposition of the secular Hamiltonian is used to calculate EPR line splitting caused by the dipole coupling. This allows calculation of operators projecting arbitrary wavefunction onto high PC eigenstates when the eigenvectors of the Hamiltonian are not known. The effective spin vectors-that is, the expectation values for vector spin operators in the PC eigenstates-are calculated. The dependence of these effective spin vectors on the external magnetic field is calculated. There is a qualitative difference between pairs having at least one integer spin (non Karmers PC) and pairs of two half-integer (Kramers PC) spins. With the help of these effective spin vectors, the dipolar lineshape of EPR lines is calculated. Analytical relations are obtained for PCs with spin S=1/2 and 1. The dependence of Pake patterns on variations of zero field splitting, Zeeman energy, temperature and dipolar coupling are illustrated.

  2. Generation of full polarization in ferromagnetic graphene with spin energy gap

    SciTech Connect

    Wu, Qing-Ping; Liu, Zheng-Fang E-mail: aixichen@ecjtu.edu.cn; Liu, Zhi-Min; Chen, Ai-Xi E-mail: aixichen@ecjtu.edu.cn; Xiao, Xian-Bo

    2014-12-22

    We propose a workable scheme for the generation of full spin polarization in ferromagnetic graphene system with strain or Rashba spin-orbit interaction. A spin energy gap can be opened in ferromagnetic graphene system in the presence of strain or Rashba spin-orbit interaction, leading to the full polarization in the spin energy gap. In addition, under the combined modulation of strain and Rashba spin-orbit interaction, the ferromagnetic graphene system can generate significantly large spin-polarized current with a full polarization in the spin energy gap. It is anticipated to apply such a phenomenon to design the electron spin devices based on the graphene.

  3. Rolling friction and energy dissipation in a spinning disc

    PubMed Central

    Ma, Daolin; Liu, Caishan; Zhao, Zhen; Zhang, Hongjian

    2014-01-01

    This paper presents the results of both experimental and theoretical investigations for the dynamics of a steel disc spinning on a horizontal rough surface. With a pair of high-speed cameras, a stereoscopic vision method is adopted to perform omnidirectional measurements for the temporal evolution of the disc's motion. The experiment data allow us to detail the dynamics of the disc, and consequently to quantify its energy. From our experimental observations, it is confirmed that rolling friction is a primary factor responsible for the dissipation of the energy. Furthermore, a mathematical model, in which the rolling friction is characterized by a resistance torque proportional to the square of precession rate, is also proposed. By employing the model, we perform qualitative analysis and numerical simulations. Both of them provide results that precisely agree with our experimental findings. PMID:25197246

  4. Spin reorientation of a nonsymmetric body with energy dissipation

    NASA Technical Reports Server (NTRS)

    Cenker, R. J.

    1973-01-01

    Stable rotating semi-rigid bodies were demonstrated analytically, and verified in flights such as Explorer 1 and ATS-5 satellites. The problem arises from the two potential orientations which the final spin vector can take after large angle reorientation from minor to major axis, i.e., along the positive or negative axis of the maximum inertia. Reorientation of a satellite initially spinning about the minor axis using an energy dissipation device may require that the final spin orientation be controlled. Examples of possible applications are the Apogee Motor Assembly with Paired Satellites (AMAPS) configuration, where proper orientation of the thruster is required; and reorientation of ATS-5, where the spin sensitive nature of the despin device (yo-yo mechanism) requires that the final spin vector point is a specified direction.

  5. Highly Efficient Room Temperature Spin Injection Using Spin Filtering in MgO

    NASA Astrophysics Data System (ADS)

    Jiang, Xin

    2007-03-01

    Efficient electrical spin injection into GaAs/AlGaAs quantum well structures was demonstrated using CoFe/MgO tunnel spin injectors at room temperature. The spin polarization of the injected electron current was inferred from the circular polarization of electroluminescence from the quantum well. Polarization values as high as 57% at 100 K and 47% at 290 K were obtained in a perpendicular magnetic field of 5 Tesla. The interface between the tunnel spin injector and the GaAs interface remained stable even after thermal annealing at 400 ^oC. The temperature dependence of the electron-hole recombination time and the electron spin relaxation time in the quantum well was measured using time-resolved optical techniques. By taking into account of these properties of the quantum well, the intrinsic spin injection efficiency can be deduced. We conclude that the efficiency of spin injection from a CoFe/MgO spin injector is nearly independent of temperature and, moreover, is highly efficient with an efficiency of ˜ 70% for the temperature range studied (10 K to room temperature). Tunnel spin injectors are thus highly promising components of future semiconductor spintronic devices. Collaborators: Roger Wang^1, 3, Gian Salis^2, Robert Shelby^1, Roger Macfarlane^1, Seth Bank^3, Glenn Solomon^3, James Harris^3, Stuart S. P. Parkin^1 ^1 IBM Almaden Research Center, San Jose, CA 95120 ^2 IBM Zurich Research Laboratory, S"aumerstrasse 4, 8803 R"uschlikon, Switzerland ^3 Solid States and Photonics Laboratory, Stanford University, Stanford, CA 94305

  6. Nucleon Spin Structure at Low Energies

    SciTech Connect

    Krebs, H.; Bernard, V.; Meissner, Ulf-G.

    2009-07-27

    We apply chiral effective field theory with explicit DELTA-1232) degrees of freedom to study double virtual Compton scattering at the photon point. Generalized spin polarizabilities are calculated up to order epsilon{sup 3} in the covariant small scale expansion. Systematic inclusion of DELTA degrees of freedom drastically improves the theoretical predictions.

  7. High-spin yrast structure of {sup 159}Ho

    SciTech Connect

    Ollier, J.; Simpson, J.; Riley, M. A.; Wang, X.; Aguilar, A.; Teal, C.; Paul, E. S.; Nolan, P. J.; Petri, M.; Rigby, S. V.; Thomson, J.; Unsworth, C.; Carpenter, M. P.; Janssens, R. V. F.; Lauritsen, T.; Zhu, S.; Darby, I. G.; Hartley, D. J.; Kondev, F. G.

    2011-08-15

    An investigation of the yrast structure of the odd-Z {sup 159}Ho nucleus to high spin has been performed. The {sup 159}Ho nucleus was populated by the reaction {sup 116}Cd({sup 48}Ca,p4n{gamma}) at a beam energy of 215 MeV, and resulting {gamma} decays were detected by the Gammasphere spectrometer. The h{sub 11/2} yrast band has been significantly extended up to I{sup {pi}=}75/2{sup -} (tentatively 79/2{sup -}). A lower frequency limit for the second (h{sub 11/2}){sup 2} proton alignment was extracted consistent with the systematics of this alignment frequency, indicating an increased deformation with neutron number in the Ho isotopes. The energy-level splitting between the signature partners in the h{sub 11/2} structures of the Ho isotopes and the neighboring N=92 isotones is discussed.

  8. In-beam spectroscopy of medium- and high-spin states in 133Ce

    NASA Astrophysics Data System (ADS)

    Ayangeakaa, A. D.; Garg, U.; Petrache, C. M.; Guo, S.; Zhao, P. W.; Matta, J. T.; Nayak, B. K.; Patel, D.; Janssens, R. V. F.; Carpenter, M. P.; Chiara, C. J.; Kondev, F. G.; Lauritsen, T.; Seweryniak, D.; Zhu, S.; Ghugre, S. S.; Palit, R.

    2016-05-01

    Medium and high-spin states in 133Ce were investigated using the 116Cd(22Ne, 5 n ) reaction and the Gammasphere array. The level scheme was extended up to an excitation energy of ˜22.8 MeV and spin 93/2 ℏ . Eleven bands of quadrupole transitions and two new dipole bands are identified. The connections to low-lying states of the previously known, high-spin triaxial bands were firmly established, thus fixing the excitation energy and, in many cases, the spin parity of the levels. Based on comparisons with cranked Nilsson-Strutinsky calculations and tilted axis cranking covariant density functional theory, it is shown that all observed bands are characterized by pronounced triaxiality. Competing multiquasiparticle configurations are found to contribute to a rich variety of collective phenomena in this nucleus.

  9. Spin-neurons: A possible path to energy-efficient neuromorphic computers

    NASA Astrophysics Data System (ADS)

    Sharad, Mrigank; Fan, Deliang; Roy, Kaushik

    2013-12-01

    Recent years have witnessed growing interest in the field of brain-inspired computing based on neural-network architectures. In order to translate the related algorithmic models into powerful, yet energy-efficient cognitive-computing hardware, computing-devices beyond CMOS may need to be explored. The suitability of such devices to this field of computing would strongly depend upon how closely their physical characteristics match with the essential computing primitives employed in such models. In this work, we discuss the rationale of applying emerging spin-torque devices for bio-inspired computing. Recent spin-torque experiments have shown the path to low-current, low-voltage, and high-speed magnetization switching in nano-scale magnetic devices. Such magneto-metallic, current-mode spin-torque switches can mimic the analog summing and "thresholding" operation of an artificial neuron with high energy-efficiency. Comparison with CMOS-based analog circuit-model of a neuron shows that "spin-neurons" (spin based circuit model of neurons) can achieve more than two orders of magnitude lower energy and beyond three orders of magnitude reduction in energy-delay product. The application of spin-neurons can therefore be an attractive option for neuromorphic computers of future.

  10. Spin-neurons: A possible path to energy-efficient neuromorphic computers

    SciTech Connect

    Sharad, Mrigank; Fan, Deliang; Roy, Kaushik

    2013-12-21

    Recent years have witnessed growing interest in the field of brain-inspired computing based on neural-network architectures. In order to translate the related algorithmic models into powerful, yet energy-efficient cognitive-computing hardware, computing-devices beyond CMOS may need to be explored. The suitability of such devices to this field of computing would strongly depend upon how closely their physical characteristics match with the essential computing primitives employed in such models. In this work, we discuss the rationale of applying emerging spin-torque devices for bio-inspired computing. Recent spin-torque experiments have shown the path to low-current, low-voltage, and high-speed magnetization switching in nano-scale magnetic devices. Such magneto-metallic, current-mode spin-torque switches can mimic the analog summing and “thresholding” operation of an artificial neuron with high energy-efficiency. Comparison with CMOS-based analog circuit-model of a neuron shows that “spin-neurons” (spin based circuit model of neurons) can achieve more than two orders of magnitude lower energy and beyond three orders of magnitude reduction in energy-delay product. The application of spin-neurons can therefore be an attractive option for neuromorphic computers of future.

  11. High-spin nuclear structure studies with radioactive ion beams

    SciTech Connect

    Baktash, C.

    1992-12-31

    Two important developments in the sixties, namely the advent of heavy-ion accelerators and fabrication of Ge detectors, opened the way for the experimental studies of nuclear properties at high angular momentum. Addition of a new degree of freedom, namely spin, made it possible to observe such fascinating phenomena as occurrences and coexistence of a variety of novel shapes, rise, fall and occasionally rebirth of nuclear collectivity, and disappearance of pairing correlations. Today, with the promise of development of radioactive ion beams (RIB) and construction of the third-generation Ge-detection systems (GAMMASPHERE and EUROBALL), the authors are poised to explore new and equally fascinating phenomena that have been hitherto inaccessible. With the addition of yet another dimension, namely the isospin, they will be able to observe and verify predictions for exotic shapes as varied as rigid triaxiality, hyperdeformation and triaxial octupole shapes, or to investigate the T = 0 pairing correlations. In this paper, they shall review, separately for neutron-deficient and neutron-rich nuclei, these and a few other new high-spin physics opportunities that may be realized with RIB. Following this discussion, they shall present a list of the beam species, intensities and energies that are needed to fulfill these goals. The paper will conclude with a description of the experimental techniques and instrumentations that are required for these studies.

  12. Adapting a compact Mott spin polarimeter to a large commercial electron energy analyzer for spin-polarized electron spectroscopy

    NASA Astrophysics Data System (ADS)

    Huang, Di-Jing; Lee, Jae-Yong; Suen, Jih-Shih; Mulhollan, G. A.; Andrews, A. B.; Erskine, J. L.

    1993-12-01

    A modified Rice University-type compact Mott spin polarimeter operating at 20 kV is adapted to a large commerical hemispherical electron energy analyzer. Normal energy analyzer functions are preserved via a retractable channeltron in the polarimeter acceleration column. In the spin-detection mode, the polarimeter permits analysis of two orthogonal transverse spin-polarization components. Electron trajectory analysis is used to optimize polarimeter lens column voltages in both normal and spin-detection modes. Performance levels are established by experiments and significantly improved spin-detection efficiency is shown to be accessible by changes in the polarimeter collection solid angle.

  13. Properties of nuclei at high spins. [A = 160 to 166

    SciTech Connect

    Stephens, F.S.

    1982-10-01

    Nuclei generate high spins by two methods, alignment of single particle angular momentum and collective rotation. The competition of these two modes is discussed for the highest spins 40 less than or equal to I less than or equal to 65 h bar. Evidence is presented that alignment of the h/sub 9/2/ and i/sub 13/2/ proton orbitals from the next higher major shell produces large affects at high spins in rotational nuclei in the A = 160-166 region. It is suggested that such major shell effects produce the still larger irregularities known to occur in the lighter nuclei of this region.

  14. High-spin states in odd-odd 168Tm

    SciTech Connect

    Cardona, M. A.; Hojman, D.; Davidson, J.; Davidson, M.; Kreiner, A. J.; Bazzacco, D.; Lenzi, S. M.; Rossi Alvarez, C.; Blasi, N.; Debray, M. E.; Levinton, G.; Marti, G.; De Poli, M.; Napoli, D. R.; Lo Bianco, G.

    2007-02-12

    High-spin states in 168Tm were investigated by means of {gamma}-ray spectroscopy techniques using the GASP multidetector array. Rotational bands have been established and identified in terms of their configurations.

  15. Energy dynamics in the Heisenberg-Kitaev spin chain

    NASA Astrophysics Data System (ADS)

    Steinigeweg, Robin; Brenig, Wolfram

    2016-06-01

    We study the Heisenberg-Kitaev spin chain in order to uncover the interplay between two qualitatively different integrable points in the physics of heat transport in one dimension. Focusing on high temperatures and using analytical as well as numerical approaches within linear response theory, we explore several directions in parameter space including exchange-coupling ratios, anisotropies, and external magnetic fields. We show the emergence of purely ballistic energy transport at all integrable points, manifest in pronounced Drude weights and low-frequency suppression of regular-conductivity contributions. Moreover, off integrability, we find extended quantum chaotic regions with vanishing Drude weights and well-defined dc conductivities. In the vicinity of the Kitaev point, we observe clear signatures of the topological gap in the response function. This gap coexists with a nonzero Drude weight in the Kitaev chain.

  16. SU(2s+1) symmetry and nonlinear dynamics of high spin magnets

    SciTech Connect

    Kovalevsky, M.Y. Glushchenko, A.V.

    2014-10-15

    The article is devoted to the description of dynamics of magnets with arbitrary spin on the basis of the Hamiltonian formalism. The relationship of quantum states and magnetic degrees of freedom has been considered. Subalgebras of Poisson bracket of magnetic values for spin s=1/2; 1; 3/2 have been established. We have obtained non-linear dynamic equations for the normal and degenerate non-equilibrium states of high-spin magnets with the SO(3), SU(4), SU(2)×SU(2), SU(3), SO(4), SO(5) symmetries of exchange interaction. The connection between models of magnetic exchange energy and the Casimir invariants has been discussed.

  17. High-spin structure of 95Pd

    NASA Astrophysics Data System (ADS)

    Mărginean, R.; Rusu, C.; Mărginean, N.; Bucurescu, D.; Ur, C. A.; de Angelis, G.; Axiotis, M.; Bazzacco, D.; Farnea, E.; Gadea, A.; Ionescu-Bujor, M.; Iordăchescu, A.; Krolas, W.; Kröll, Th.; Lenzi, S. M.; Lunardi, S.; Napoli, D. R.; Alvarez, C. Rossi; Wrzesinski, J.

    2012-09-01

    The level scheme of the neutron-deficient nucleus 95Pd has been studied with the 58Ni + 40Ca fusion-evaporation reaction at 135 MeV with the GASP γ-ray array, the ISIS silicon ball, and the N-ring neutron detector. Excited levels with spins at least up to (45)/(2)ℏ are reported for both parities. The observed experimental data are compared to large-scale shell-model calculations.

  18. (Medium energy spin physics with lasers)

    SciTech Connect

    Cates, G.D.

    1992-01-01

    During the first two years of this program, we have successfully investigated two new methods for the production of polarized muonic helium. This work was done at LAMPF in collarboration with a group from Syracuse University. Traditionally, polarized muonic helium has been formed by stopping polarized muons in unpolarized atoms. Unfortunately, because of depolarization in the muon cascade to the ground state, residual polarizations are only {approximately}3%. The two methods we have developed both achieve much higher muon polarizations. To accomplish our goals, we first developed an appropriate muon beam for use with our small gas targets. During the summer of 1990, we stopped unpolarized negative muons in nuclear polarized {sup 3}He. The muons were polarized in the cascade to the ground state through the hyperfine interaction with the nucleus. The resulting muon polarizations were 7.2 {plus minus} 0.8% for a 100% nuclear polarized target. While higher polarizations are clearly desirable for practical purposes, this experiment yielded important insights on spin interactions that occur in muonic atoms. Also, the ability to rapidly reverse the target polarization gave the experiment good sensitivity with minimal systematic effects. Last summer, we completed an experiment in which we polarized muonic helium by direct spin interaction with an optically pumped Rb vapor. In this technique, the muonic helium atom is polarized through a combination of charge exchange and spin exchange with the polarized valence electron of the Rb vapor. In contrast to the technique described in appendix A, the {sup 3}He nuclei are not polarized. This last technique yielded dramatic polarizations approaching 50%.

  19. High-resolution spin-polarized scanning electron microscopy (spin SEM).

    PubMed

    Kohashi, Teruo; Konoto, Makoto; Koike, Kazuyuki

    2010-01-01

    We have developed spin-polarized scanning electron microscopy (spin SEM) with a 5-nm resolution. The secondary electron optics is very important, as it needs to transfer a sufficient number of secondary electrons to the spin polarimeter, due to the low efficiency of the polarimeter. The optics was designed using a three-dimensional (3D) simulation program of the secondary electron trajectories, and it achieves highly efficient collection and transport of the secondary electrons even though the distance between the sample and the objective lens exit of the electron gun remains short. Moreover, the designed optics enables us to obtain clear SEM images in the spin SEM measurement and to precisely adjust the probe beam shape. These functions lead to images with high spatial resolution and sufficient signal-to-noise (S/N) ratios. This optics has been installed in an ultra-high vacuum (UHV) spin SEM chamber with a Schottky-type electron gun for the probe electron beam. We observed recorded bits on a perpendicular magnetic recording medium and visualized small irregularities in the bit shapes around the track edges and bit boundaries. The high resolution of 5 nm was demonstrated by observing the smallest domain composed by a single grain in the recording medium. PMID:19840986

  20. Investigation of High-Spin States in ^203Rn

    NASA Astrophysics Data System (ADS)

    Beausang, C. W.; Novak, J. R.; Caprio, M.; Casten, R. F.; Cederkall, J.; Cooper, J. R.; Krücken, R.; Wang, Z.; Zamfir, N. V.; Barton, C. J.

    1999-10-01

    High-spin states in ^203Rn were populated following the reaction ^34S + ^174Yb + 5n at beam energies ranging from 160 to 170 MeV. Gamma-rays were detected using the multi-Ge detector array YRAST Ball located at the Wright Nuclear Structure Laboratory. In addition the SCARY array, an array of 28 solar cell detectors, each 1 cm by 1 cm, was arranged around the target at backward angles. These were used to detect fission fragments and hence discriminate against the very large fission background encountered in this reaction. Following our excitation function measurement several transitions can be assigned to ^203Rn, where previously no information was available on excited states. Data analysis is continuing and preliminary results will be presented. This work is supported by the US-DOE under grant number DE-FG02-91ER-40609.

  1. Normal-Deformed High-Spin States in ^81Sr

    NASA Astrophysics Data System (ADS)

    Birriel, I.; Winchell, D. F.; Saladin, J. X.; Cristancho, F.; Landulfo, E.; Wood, V. Q.; Baktash, C.; Brinkman, M. J.; Gross, C. J.; Jin, H.-Q.; Rudolph, D.; Stracener, D. W.; Yu, C.-H.; Devlin, M.; Hua, P.-F.; Korolija, M.; Lafosse, D. R.; Lerma, F.; Sarantites, D. G.; Döring, J.; Sylvan, G.; Tabor, S.; Cederwall, B.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Maier, M. R.; Rathbun, W.; Vander Mollen, A.; Werner, T. R.

    1998-04-01

    Normal-deformed high-spin states in ^81Sr were populated with the reactions ^58Ni(^29Si,α2p) and ^58Ni(^28Si,4p) with beam energies of 128 and 130 MeV, respectively, from the 88-inch cyclotron at LBNL. Gamma rays from the reactions were detected with Gammasphere, and evaporated α particles and protons were detected with Microball. Our results are consistent with previous work (D.H. Smalley et al, Nucl. Phys. A611 (1996) 96). In addition, two new negative parity rotational bands (built on a 295-241 keV cascade(S.E. Arnell et al, J.Phys. G9, (1983) 1217)) and 11 new side bands have been found. In all, the level scheme has been extended by 65 new states, along with 78 new transitions. The results will be discussed in the framework of the cranked shell model.

  2. High-spin level scheme of {sup 183}Au

    SciTech Connect

    Song, L.T.; Zhou, X.H.; Zhang, Y. H.; Guo, Y. X.; Lei, X.G.; Zheng, Y.; Liu, M.L.; De Angelis, G.; Marginean, N.; Gadea, A.; Napoli, D.R.; Axiotis, M.; Rusu, C.; Martinez, T.

    2005-01-01

    High-spin states in {sup 183}Au have been studied experimentally using the {sup 159}Tb({sup 29}Si,5n){sup 183}Au reaction at a beam energy of 140 MeV. Three- or higherfold {gamma}-ray coincidences have been measured using the detector array of GASP. The level scheme of {sup 183}Au was revised and extended. A rotational band proposed as the unfavored signature branch of the {pi}i{sub 13/2} band has been observed for {sup 183}Au. Interaction properties between the two negative-signature bands of the {pi}h{sub 9/2}-{pi}f{sub 7/2} system have been discussed for the light odd-A Au nuclei.

  3. Magnetic relaxation of high spin magnetic molecules

    NASA Astrophysics Data System (ADS)

    Luo, Nie

    The magnetic relaxation phenomena in Mn12 and the physics underlining these experiment results are investigated in this dissertation. We give a review on currently available theories to account for the spin or paramagnetic relaxation occurring in this system. Density matrix formalism is used to investigate the general problem of a system interacting with a bath of thermal equilibrium phonons, which gives a set of rate equations. Numerical solutions to the rate equations are also carried out. Finally comparisons between the theory and the experimentals are made to show the merits and deficiencies of the theoretical approach that we have adopted.

  4. Existence of an exotic torus configuration in high-spin excited states of 40Ca.

    PubMed

    Ichikawa, T; Maruhn, J A; Itagaki, N; Matsuyanagi, K; Reinhard, P-G; Ohkubo, S

    2012-12-01

    We investigate the possibility of the existence of the exotic torus configuration in the high-spin excited states of (40)Ca. We here consider the spin alignments about the symmetry axis. To this end, we use a three-dimensional cranked Skyrme Hartree-Fock method and search for stable single-particle configurations. We find one stable state with the torus configuration at the total angular momentum J=60 ħ and an excitation energy of about 170 MeV in all calculations using various Skyrme interactions. The total angular momentum J=60 ħ consists of aligned 12 nucleons with the orbital angular momenta Λ=+4, +5, and +6 for spin-up or -down neutrons and protons. The obtained results strongly suggest that a macroscopic amount of circulating current breaking the time-reversal symmetry emerges in the high-spin excited state of (40)Ca. PMID:23368188

  5. Fission Barrier of ^254No at High Spin

    NASA Astrophysics Data System (ADS)

    Henning, G.; Khoo, T. L.; Seweryniak, D.; Back, B. B.; Bertone, P. F.; Carpenter, M. P.; Greene, J. P.; Gürdal, G.; Hoffman, C. R.; Janssens, R. V. F.; Kay, B. P.; Kondev, F. G.; Lauritsen, T.; Lister, C. J.; McCutchan, E. A.; Nair, C.; Rogers, A. M.; Zhu, S.; Chiara, C. J.; Hauschild, K.; Lopez-Martens, A.; Heinz, A.; Piot, J.; Chowdhury, P.; Lakshmi, S.

    2010-11-01

    Superheavy nuclei provide opportunities to study nuclear structure at the limits in charge, spin and excitation energy. These nuclei exist only because shell effects create a fission barrier Bf. Hence, it is important to determine Bf and its spin dependence. For ^254No, the maximum spin and energy were found [1] to be Imax= 22 and E* = 8 MeV in the reaction ^208Pb(^48Ca,2n) at a beam energy of 219 MeV. At 223 MeV, the maximum spin increases to 32. In contrast, the spin in ^220Th, produced [2] in the ^176Yb(^48 Ca,4n) reaction at 206 and 219 MeV, saturates at 20. A measurement of the entry distribution of ^254No at 223 MeV has been performed to determine Bf(I) and results will be reported.[4pt] [1] P. Reiter et al., Phys. Rev. Lett. 84, 3542 (2000).[0pt] [2] A. Heinz et al., Nucl. Phys. A682, 458c (2001)

  6. Low energy spin dynamics in the spin ice, Ho2Sn2O7

    SciTech Connect

    Ehlers, Georg; Huq, Ashfia; Diallo, Souleymane Omar; Adriano, Cris; Rule, K; Cornelius, A. L.; Fouquet, Peter; Pagliuso, P G; Gardner, Jason

    2012-01-01

    The magnetic properties of Ho{sub 2}Sn{sub 2}O{sub 7} have been investigated and compared to other spin ice compounds. Although the lattice has expanded by 3% relative to the better studied Ho{sub 2}Ti{sub 2}O{sub 7} spin ice, no significant changes were observed in the high temperature properties, T {approx}> 20 K. As the temperature is lowered and correlations develop, Ho{sub 2}Sn{sub 2}O{sub 7} enters its quantum phase at a slightly higher temperature than Ho{sub 2}Ti{sub 2}O{sub 7} and is more antiferromagnetic in character. Below 80 K a weak inelastic mode associated with the holmium nuclear spin system has been measured. The hyperfine field at the holmium nucleus was found to be {approx}700 T.

  7. Elastic anomalies and phonon damping in a metallic high spin-low spin system

    NASA Astrophysics Data System (ADS)

    Ihlemann, J.; Bärner, K.

    1984-12-01

    The elastic constants and the sound attenuation in single crystals of the metallic high spin (hs)-low spin (ls) system MnAs 1- xP x have been measured for temperaturres between 10 and 500 K. Elastic anomalies and damping maxima have been found for the second-order displacive (B8 1⇌B31) phase transition, the hs-ls transition and for the magnetic order-disorder transition. The phenomena near the hs-ls transition, in particular, are interpreted in terms of a condensation of a soft static phonon at the ls (hs) site in a hs (ls) matrix.

  8. New high spin states and isomers in the {sup 208}Pb and {sup 207}Pb nuclei

    SciTech Connect

    Broda, R.; Wrzesinski, J.; Pawlat, T.

    1996-12-31

    The two most prominent examples of the heavy doubly closed shell (DCS) nuclei, {sup 208}Pb and {sup 132}Sn, are not accessible by conventional heavy-ion fusion processes populating high-spin states. This experimental difficulty obscured for a long time the investigation of yrast high-spin states in both DCS and neighboring nuclei and consequently restricted the study of the shell model in its most attractive regions. Recent technical development of multidetector gamma arrays opened new ways to exploit more complex nuclear processes which populate the nuclei of interest with suitable yields for gamma spectroscopy and involve population of moderately high spin states. This new possibility extended the range of accessible spin values and is a promising way to reach new yrast states. Some of these states are expected to be of high configurational purity and can be a source of important shell model parameters which possibly can be used later to check the validity of the spherical shell model description at yet higher spin and higher excitation energy. The nuclei in the closest vicinity of {sup 132}Sn are produced in spontaneous fission and states with spin values up to I=14 can be reached in fission gamma spectroscopy studies with the presently achieved sensitivity of gamma arrays. New results on yrast states in the {sup 134}Te and {sup 135}I nuclei populated in fission of the {sup 248}Cm presented at this conference illustrate such application of the resolving power offered by modern gamma techniques.

  9. Velocity of the high-spin low-spin interface inside the thermal hysteresis loop of a spin-crossover crystal, via photothermal control of the interface motion.

    PubMed

    Slimani, Ahmed; Varret, François; Boukheddaden, Kamel; Garrot, Damien; Oubouchou, Hassane; Kaizaki, Sumio

    2013-02-22

    We investigated by optical microscopy the thermal transition of the spin-crossover dinuclear iron(II) compound [(Fe(NCSe)(py)(2))(2)(m-bpypz)]. In a high-quality crystal the high-spin (HS) low-spin (LS) thermal transition took place with a sizable hysteresis, at ~108 K and ~116 K on cooling and heating, respectively, through the growth of a single macroscopic domain with a straight LS and HS interface. The interface orientation was almost constant and its propagation velocity was close to ~6 and 26 μ m s(-1) for the on-cooling and on-heating processes, respectively. We found that the motion of the interface was sensitive to the intensity of the irradiation beam of the microscope, through a photothermal effect. By fine-tuning the intensity we could stop and even reverse the interface motion. This way we stabilized a biphasic state of the crystal, and we followed the spontaneous motion of the interface at different temperatures inside the thermal hysteresis loop. This experiment gives access for the first time to an accurate determination of the equilibrium temperature in the case of thermal hysteresis--which was not accessible by the usual quasistatic investigations. The temperature dependence of the propagation velocity inside the hysteretic interval was revealed to be highly nonlinear, and it was quantitatively reproduced by a dynamical mean-field theory, which made possible an estimate of the macroscopic energy barrier. PMID:23473199

  10. Energy transport between two integrable spin chains

    NASA Astrophysics Data System (ADS)

    Biella, Alberto; De Luca, Andrea; Viti, Jacopo; Rossini, Davide; Mazza, Leonardo; Fazio, Rosario

    2016-05-01

    We study the energy transport in a system of two half-infinite XXZ chains initially kept separated at different temperatures, and later connected and let free to evolve unitarily. By changing independently the parameters of the two halves, we highlight, through bosonization and time-dependent matrix-product-state simulations, the different contributions of low-lying bosonic modes and of fermionic quasiparticles to the energy transport. In the simulations we also observe that the energy current reaches a finite value which only slowly decays to zero. The general picture that emerges is the following. Since integrability is only locally broken in this model, a preequilibration behavior may appear. In particular, when the sound velocities of the bosonic modes of the two halves match, the low-temperature energy current is almost stationary and described by a formula with a nonuniversal prefactor interpreted as a transmission coefficient. Thermalization, characterized by the absence of any energy flow, occurs only on longer time scales which are not accessible with our numerics.

  11. An overview of spin physics

    SciTech Connect

    Prescott, C.Y.

    1991-07-01

    Spin physics is playing an increasingly important role in high energy experiments and theory. This review looks at selected topics in high energy spin physics that were discussed at the 9th International Symposium on High Energy Spin Physics at Bonn in September 1990.

  12. Applications of highly spin-polarized xenon in NMR

    SciTech Connect

    Long, H.W. |

    1993-09-01

    The main goal of the work presented in this thesis is produce highly spin-polarized xenon to create much greater signal intensities (up to 54,000 times greater) so as to allow studies to be made on systems with low surface area and long spin-lattice relaxation times. The spin-exchange optical pumping technique used to create high nuclear spin polarization is described in detail in chapter two. This technique is initially applied to some multiple-pulse optically detected NMR experiments in low magnetic field (50G) that allow the study of quadrupoler interactions with a surface of only a few square centimeters. In chapter three the apparatus used to allow high field {sup 129}Xe NMR studies to be performed with extremely high sensitivity is described and applied to experiments on diamagnetic susceptibility effects in thin ({approximately}2000 layers) films of frozen xenon. Preliminary surface investigations of laser polarized {sup 129}Xe adsorbed an a variety of materials (salts, molecular crystals, amorphous carbon, graphite) are then discussed. A full detailed study of the surface of a particular polymer, poly(acrylic acid), is presented in chapter four which shows the kind of detailed information that can be obtained from this technique. Along with preliminary results for several similar polymers, a summary is given of xenon studies of a novel ultra-high surface area polymer, poly(triarylcarbinol). Finally in chapter five the exciting possibility of transferring the high spin order of the laser polarized xenon has been used to transfer nuclear spin order to {sup 13}CO{sub 2} in a xenon matrix and to protons on poly(triarylcarbinol).

  13. Spin injection into multilayer graphene from highly spin-polarized Co2FeSi Heusler alloy

    NASA Astrophysics Data System (ADS)

    Yamaguchi, Takehiro; Moriya, Rai; Oki, Soichiro; Yamada, Shinya; Masubuchi, Satoru; Hamaya, Kohei; Machida, Tomoki

    2016-06-01

    We demonstrate electrical spin injection into multilayer graphene (MLG) in a lateral spin valve device from a highly spin-polarized Co2FeSi (CFS) Huesler electrode. Exfoliated MLG was transferred onto prepatterned epitaxial CFS wires grown on an Si(111) substrate by a polymer-based transfer method. This method enabled us to fabricate multiple single-crystal CFS electrodes in contact with MLG. Electrical spin injection from CFS to MLG was detected through nonlocal magnetoresistance (MR) measurement. A nonlocal spin signal of 430 Ω was observed; this is the largest value among all reported nonlocal MR values in graphene-based devices.

  14. Composite Fermion Spin Polarization Energy with Finite Layer Thickness

    NASA Astrophysics Data System (ADS)

    Shayegan, Mansour; Liu, Yang; Hasdemir, Sukret; Pfeiffer, Loren; West, Ken; Baldwin, Kirk

    2014-03-01

    We study the spin polarization transitions of fractional quantum Hall (FQH) states in the filling range 1 < ν < 2 in symmetric quantum wells (QWs), as a function of density. Our results reveal a strong well-width dependence of the critical density nC and ratio between the Zeeman energy (EZ) normalized to the Coulomb energy (e2 / 4 πɛlB), above which a certain FQH state becomes spin polarized. For example, the ν = 7 / 5 FQH state becomes spin polarized at about 3 times higher density or 1.7 times larger EZ in the 31-nm-wide QW than in the 65-nm-wide QW. This well-width dependence of the spin polarization stems from by the finite electron layer thickness in these QWs and the resulting softening of the Coulomb interaction. We acknowledge support through the DOE BES (DE-FG02-00-ER45841) for measurements, and the Gordon and Betty Moore Foundation (Grant GBMF2719), Keck Foundation, and the NSF (DMR-0904117, DMR-1305691 and MRSEC DMR-0819860) for sample fabrication. Work at Arg.

  15. Observation of a highly spin-polarized topological surface state in GeBi2Te4

    NASA Astrophysics Data System (ADS)

    Okamoto, K.; Kuroda, K.; Miyahara, H.; Miyamoto, K.; Okuda, T.; Aliev, Z. S.; Babanly, M. B.; Amiraslanov, I. R.; Shimada, K.; Namatame, H.; Taniguchi, M.; Samorokov, D. A.; Menshchikova, T. V.; Chulkov, E. V.; Kimura, A.

    2012-11-01

    Spin polarization of a topological surface state for GeBi2Te4, the newly discovered three-dimensional topological insulator, has been studied by means of state-of-the-art spin- and angle-resolved photoemission spectroscopy. It has been revealed that the disorder in the crystal has a minor effect on the surface-state spin polarization, which is 70% near the Dirac point in the bulk energy gap region (˜180 meV). This finding promises not only to realize a highly spin-polarized surface-isolated transport but also to add functionality to its thermoelectric and thermomagnetic properties.

  16. Shape evolution at high spin states in Kr and Br isotopes

    SciTech Connect

    Trivedi, T.; Palit, R.; Naik, Z.; Jain, H. C.; Negi, D.; Kumar, R.; Singh, R. P.; Muralithar, S.; Pancholi, S. C.; Bhowmik, R. K.; Yang, Y.-C.; Sun, Y.; Sheikh, J. A.; Raja, M. K.; Kumar, S.; Choudhury, D.; Jain, A. K.; Mehrotra, I.

    2014-08-14

    The high spin states in A = 75, Kr and Br isotopes have been populated via fusion-evaporation reaction at an incident beam energy of 90 MeV. The de-exciting γ-rays were detected utilizing the Indian National Gamma Array (INGA). Lifetime of these excited high spin states were determined by Doppler-shift attenuation method. Experimental results obtained from lifetime measurement are interpreted in the frame work of projected shell-model to get better insight into the evolution of collectivity. Comparison of the calculations of the model with transitional quadrupole moments Q{sub t} of the positive and negative parity bands firmly established their configurations.

  17. Energy Scaling of Spin Tune due to RHIC Snakes

    SciTech Connect

    MacKay,W.W.

    2009-01-02

    For a ring like RHIC with two full Siberian snakes on opposite sides of the ring, the spin tune for a flat orbit will be 1/2 if the snake rotation axes are perpendicular, {Delta}{phi} = {phi}{sub 9}-{phi}{sub 3} = {pi}/2. Here {phi}{sup 9} and {phi}{sub 3} are respectively the direction of the rotation axes of the 9 o'clock and 3 o'clock snakes relative to the design trajectory as shown in Figure 1. If the two snakes are slightly detuned by the same amount such that the rotation axes are no longer perpendicular, then the deviation of the closed-orbit spin tune {nu}{sub 0} from 1/2 is given by {Delta}{nu}{sub 0} {approx_equal} ({Delta}{mu}){sup 2}/4{pi} cosG{gamma}{pi} - 2{Delta}{phi}/{pi} {approx_equal} 2{Delta}{phi}/180{sup o} with G{gamma} at a half integer, and where {Delta}{mu} is the deviation of snake rotation angle from 180{sup o}. It should be noted that there is a sign ambiguity in {Delta}{mu}{sub 0} since a spin tune of 0.495 is also a spin tune of 0.505, depending on the direction taken along the stable spin axis. In order to understand the effect of energy scaling on the snake axis direction, I have integrated the trajectory and spin rotation through a model of a RHIC snake (bi9-snk7) and found the energy (U) dependence of the snake axis angle {phi}{sub 9} and rotation angle {mu} as shown. A {approx_equal} p{sup -2} scaling of errors is typical in helical snakes. To first order, the orbit excursion drops as p{sup -1} and the spin precessions about transverse fields increase as {gamma} giving an approximate cancellation with energy, so we do not expect much change during the field ramp. The next order term which comes in is primarily proportional to p{sup -2}; although naively one might expect a slight effect inversely proportional to the velocity since {gamma}/p {proportional_to} c/{nu} {approx_equal} 1 + 1/2{gamma}{sup 2}.

  18. Tunable bistable devices for harvesting energy from spinning wheels

    NASA Astrophysics Data System (ADS)

    Elhadidi, Mohamed; Helal, Mohammed; Nassar, Omar; Arafa, Mustafa; Zeyada, Yasser

    2015-04-01

    Bistable systems have recently been employed for vibration energy harvesting owing to their favorable dynamic characteristics and desirable response for wideband excitation. In this paper, we investigate the use of bistable harvesters to extract energy from spinning wheels. The proposed harvester consists of a piezoelectric cantilever beam that is mounted on a rigid spinning hub and carries a tip mass in the form of a permanent magnet. Magnetic repulsion forces from an opposite magnet cause the beam to possess two stable equilibrium positions. Inter-well lead-lag oscillations caused by rotation in a vertical plane provide a good source for energy extraction. The design offers frequency tuning, as the centrifugal forces strain the harvester, thereby increasing its natural frequency to cope with a variable rotational speed. This has applications in self-powered sensors mounted on spinning wheels, such as tire pressure monitoring sensors. An effort is made to select the design parameters to enable the harvester to exhibit favorable inter-well oscillations across a range of rotational speeds for enhanced energy harvesting. Findings of the present work are verified both numerically and experimentally.

  19. Pulsed electron-electron double resonance spectroscopy between a high-spin Mn(2+) ion and a nitroxide spin label.

    PubMed

    Akhmetzyanov, D; Plackmeyer, J; Endeward, B; Denysenkov, V; Prisner, T F

    2015-03-14

    Pulsed Electron-Electron Double Resonance (PELDOR) has attracted considerable attention for biomolecular applications, as it affords precise measurements of distances between pairs of spin labels in the range of 1.5-8 nm. Usually nitroxide moieties incorporated by site-directed spin labelling with cysteine residues are used as spin probes in protein systems. Recently, naturally occurring cofactors and metal ions have also been explored as paramagnetic spin species for such measurements. In this work we investigate the performance of PELDOR between a nitroxide spin label and a high-spin Mn(2+) ion in a synthetic model compound at Q-band (34 GHz) and G-band (180 GHz). We demonstrate that the distances obtained with high-frequency PELDOR are in good agreement with structural predictions. At Q-band frequencies experiments have been performed by probing either the high-spin Mn(2+) ion or the nitroxide spin label. At G-band frequencies we have been able to detect changes in the dipolar oscillation frequency, depending on the pump-probe positions across the g-tensor resolved nitroxide EPR spectrum. These changes result from the restricted mobility of the nitroxide spin label in the model compound. Our results demonstrate that the high-spin Mn(2+) ion can be used for precise distance measurements and open the doors for many biological applications, as naturally occurring Mg(2+) sites can be readily exchanged for Mn(2+). PMID:25669744

  20. Entanglement in the XX spin chain with an energy current

    SciTech Connect

    Eisler, V.

    2005-04-01

    We consider the ground state of an XX chain that is constrained to carry a current of energy. The von Neumann entropy of a block of L neighboring spins, describing entanglement of the block with the rest of the chain, is computed. Recent calculations have revealed that the entropy in the XX model diverges logarithmically with the size of the subsystem. We show that the presence of the energy current increases the prefactor of the logarithmic growth. This result indicates that the emergence of the energy current gives rise to an increase of entanglement.

  1. Loss of collectivity in the transitional {sup 156}Er nucleus at high spin

    SciTech Connect

    Paul, E. S.; Rigby, S. V.; Choy, P. T. W.; Evans, A. O.; Nolan, P. J.; Riley, M. A.; Campbell, D. B.; Pipidis, A.; Simpson, J.; Appelbe, D. E.; Joss, D. T.; Clark, R. M.; Cromaz, M.; Fallon, P.; Goergen, A.; Lee, I. Y.; Macchiavelli, A. O.; Ward, D.; Ragnarsson, I.

    2009-04-15

    The {sup 114}Cd({sup 48}Ca,6n{gamma}) reaction at 215 MeV has been investigated using the Gammasphere spectrometer to study the high-spin structure of the nucleus {sub 68}{sup 156}Er{sub 88}. Many new transitions have been established along with definitive spin-parity level assignments from a high-fold angular-distribution analysis. In addition, absolute B(M1) and B(E1) strengths have been inferred from measured {gamma}-ray branching ratios. Strong B(E1) strength (10{sup -3} W.u.) is discussed in terms of possible octupole collectivity at low spin. At high spin, this nucleus undergoes a Coriolis-induced shape transition from a prolate state of collective rotation to a noncollective, triaxial-oblate configuration. The yrast positive-parity structure ultimately terminates in an energetically favored oblate state at I{sup {pi}}=42{sup +}. Several weak high-energy {gamma}-ray transitions have been discovered that feed this favored state. State-of-the-art cranked Nilsson-Strutinsky calculations are used to interpret the high-spin behavior of {sup 156}Er and comparisons are made with other N=88 isotones.

  2. Fe-S Bonded Interactions Involving High and Low Spin State Divalent Fe Atoms

    NASA Astrophysics Data System (ADS)

    Gibbs, G. V.; Cox, D. F.; Rosso, K. M.; Ross, N. L.

    2006-12-01

    Bond critical point and local energy density properties together with the net atomic charges were generated for the theoretical electron density distributions, ρ(r), for a variety of Fe sulfide crystalline materials with high and low spin state divalent Fe atoms in octahedral coordination and high spin state divalent and trivalent Fe atoms in tetrahedral coordination. The value of the electron density, ρ(rc), and the Laplacian, ▽ 2ρ(rc), the local potential energy density, V(rc), and the local electronic energy density, H(rc), at bond critical points, (rc), each increases and the local kinetic energy density, G(rc), decreases as the coordination numbers of the Fe atoms decrease and the shared character of the Fe-S bonds is indicated to increase. The properties of the bonded interactions involving the octahedrally coordinated low spin state divalent Fe atoms in pyrite and marcasite depart substantially from those of the octahedrally coordinated high spin state divalent Fe atoms in troilite, symthite and greigite. The Fe-S bond lengths are shorter and the values of ρ(rc) and ▽ 2ρ(rc), are larger for pyrite and marcasite indicating that the accumulation and local concentration of ρ(r) in the vicinity of rc is greater than those involving the longer, high spin state Fe-S bonded interactions. The net atomic charges conferred on the Fe and S atoms in pyrite and marcasite are also smaller than those calculated for sulfides with high spin state octahedrally coordinate divalent Fe atoms. Collectively, the Fe-S bonded interactions are indicated to be intermediate in character on the basis of their bond indices with the low spin Fe-S bonds being more shared interactions than the high spin state bonded interactions. S-S bond paths exist between each of the surface S atoms of the adjacent layers of FeS6 octahedra in smythite, indicating that the neutral Fe3S4 layers are linked together by S-S bonded interactions. Such interactions not only exist between the S atoms on

  3. Lifetimes of high-spin states in {sup 162}Yb

    SciTech Connect

    Carpenter, M.P.; Janssens, R.V.F.; Henry, R.G.

    1995-08-01

    A measurement on lifetimes of high-spin states in the yrast and near-yrast rotational bands in {sup 162}Yb was carried out at ATLAS in order to determine the evolution of collectivity as a function of angular momentum using the {sup 126}Te({sup 40}Ar,4n){sup 162}Yb reaction at 170 MeV. Previous lifetime measurements in the {sup 164,166,168}Yb isotopes showed a dramatic decrease in the transition quadrupole moment Q{sub t} with increasing spin. It was suggested that this decrease in Q{sub t} is brought about by the rotationally-induced deoccupation of high-j configurations, mainly i{sub 13/2} neutrons. If this interpretation is correct, the heavier isotopes should have a larger decrease in Q{sub t} than the lighter mass nuclides due to the position of the Fermi surface in the i{sub 13/2} subshell. Indeed, {sup 160}Yb does not show a clear decrease in Q{sub t} at high spin. No high spin lifetime information exists for {sup 162}Yb, thus this experiment fills the gap of measured Q{sub t}`s in the light Yb series. The data is currently being analyzed.

  4. Ultra-High Spin Spectroscopy In Er Nuclei

    NASA Astrophysics Data System (ADS)

    Simpson, J.

    2008-11-01

    The discoveries observed in the ongoing conflict between collective and single-particle nuclear behaviour with increasing angular momentum have driven the field of nuclear spectroscopy for many decades and have given rise to new nuclear phenomena. Recently a new frontier of γ spectroscopy at ultra-high spin has been opened in the rare-earth region with rotational bands that bypass the classic band-terminating states that appear at spin 45ℏ in the N 90 Er nuclei. These weakly populated rotational structures have characteristics of triaxial strongly-deformed bands. Such structures have been observed in 157,158,160Er, following a series of experiments using the Gammasphere spectrometer. These observations herald a return to collective excitations at spins of about 50 to 65ℏ. This talk reviews the status of the spectroscopy and understanding of the observed structures in these Er and neighbouring nuclei.

  5. Ultra-High Spin Spectroscopy In Er Nuclei

    SciTech Connect

    Simpson, J.

    2008-11-11

    The discoveries observed in the ongoing conflict between collective and single-particle nuclear behaviour with increasing angular momentum have driven the field of nuclear spectroscopy for many decades and have given rise to new nuclear phenomena. Recently a new frontier of {gamma} spectroscopy at ultra-high spin has been opened in the rare-earth region with rotational bands that bypass the classic band-terminating states that appear at spin 45({Dirac_h}/2{pi}) in the N 90 Er nuclei. These weakly populated rotational structures have characteristics of triaxial strongly-deformed bands. Such structures have been observed in {sup 157,158,160}Er, following a series of experiments using the Gammasphere spectrometer. These observations herald a return to collective excitations at spins of about 50 to 65({Dirac_h}/2{pi}). This talk reviews the status of the spectroscopy and understanding of the observed structures in these Er and neighbouring nuclei.

  6. Datta-and-Das spin transistor controlled by a high-frequency electromagnetic field

    NASA Astrophysics Data System (ADS)

    Sheremet, A. S.; Kibis, O. V.; Kavokin, A. V.; Shelykh, I. A.

    2016-04-01

    We developed the theory of spin dependent transport through a spin-modulator device (so-called Datta-and-Das spin transistor) in the presence of a high-frequency electromagnetic field (dressing field). Solving the Schrödinger problem for dressed electrons, we demonstrated that the field drastically modifies the spin transport. In particular, the dressing field leads to renormalization of spin-orbit coupling constants that varies conductivity of the spin transistor. The present effect paves the way for controlling the spin-polarized electron transport with light in prospective spin-optronic devices.

  7. RHIC SPIN FLIPPER

    SciTech Connect

    BAI,M.; ROSER, T.

    2007-06-25

    This paper proposes a new design of spin flipper for RHIC to obtain full spin flip with the spin tune staying at half integer. The traditional technique of using an rf dipole or solenoid as spin flipper to achieve full spin flip in the presence of full Siberian snake requires one to change the snake configuration to move the spin tune away from half integer. This is not practical for an operational high energy polarized proton collider like RHIC where beam lifetime is sensitive to small betatron tune change. The design of the new spin flipper as well as numerical simulations are presented.

  8. Imaging chiral spin textures with spin-polarized low energy electron microscopy

    NASA Astrophysics Data System (ADS)

    Schmid, Andreas

    2015-03-01

    Chirality in magnetic materials is fundamentally interesting holds potential for logic and memory applications. Using spin-polarized low-energy electron microscopy, we recently observed chiral Néel walls in thin films. We developed ways to tailor the Dzyaloshinskii-Moriya interaction, which drives the chirality, by interface engineering, and we found that Néel- and Bloch- chirality type can be tuned in the presence of uniaxial strain. This work was done in collaboration with G. Chen, A.T.N'diaye, T.P.Ma, A.Mascaraque, C.Won, Z.Q.Qiu, Y.Z.Wu.

  9. Dynamics of Rb and 21Ne spin ensembles interacting by spin exchange with a high Rb magnetic field

    NASA Astrophysics Data System (ADS)

    Fang, Jiancheng; Chen, Yao; Lu, Yan; Quan, Wei; Zou, Sheng

    2016-07-01

    We report on the dynamics of spin-polarized Rb and 21Ne ensembles in which the 21Ne spin ensemble in a glass vapor cell experiences a high magnetic field produced by a Rb electron-spin ensemble. The coupled spin ensembles are modeled and the response of the transverse-step magnetic field excitation is solved and studied experimentally. Moreover, we analyze the frequency response of the ensembles to a transverse-oscillating magnetic field. We demonstrate the strong transverse damping and large frequency shift of the 21Ne spin ensemble as the precession frequencies of 21Ne spin and Rb spin match and the magnetic resonance spectroscopies of the two ensembles merge into one. We also demonstrate the operation of the spin ensembles as a self-compensating co-magnetometer that is insensitive to low-frequency magnetic fields that would be useful for rotation rate sensing. For such sensing applications, a large Rb density is achieved to polarize the 21Ne spins. This density leads to a high Rb electron spin magnetic field and we demonstrate its effect on the dynamics of the co-magnetometer.

  10. Observations of high spin states in {sup 179}Au

    SciTech Connect

    Carpenter, M.P.; Ahmad, I.; Blumenthal, D.J.

    1995-08-01

    As part of a current study on the properties of the {pi} i{sub 13/2} intruder state in the A = 175-190 region, we conducted an experiment at ATLAS to observe high spin states in {sup 179}Au utilizing the reaction {sup 144}Sm({sup 40}Ar,p4n) at beam energies of 207 MeV and 215 MeV. To aid in the identification of {sup 179}Au, and to filter out the large amount of events from fission by-products, the Fragment Mass Analyzer was utilized in conjunction with ten Compton-suppression germanium detectors. In total, 11 x 10{sup 6} {gamma}-{gamma} and 4 x 10{sup 5} {gamma}-recoil events were collected. By comparing {gamma}-rays in coincidence with an A = 179 recoil mass gate and {gamma}-rays in coincidence with Au K{alpha} and K{beta} X-rays, ten {gamma}-rays were identified as belonging to {sup 179}Au. Based on {gamma}-ray coincidence relationships and on comparisons with neighboring odd-A Au nuclei, we constructed a tentative level scheme and assigned a rotational-like sequence to the {pi} i{sub 13/2} proton configuration.

  11. A new high-spin isomer in 195Bi

    NASA Astrophysics Data System (ADS)

    Roy, T.; Mukherjee, G.; Madhavan, N.; Rana, T. K.; Bhattacharya, Soumik; Asgar, Md. A.; Bala, I.; Basu, K.; Bhattacharjee, S. S.; Bhattacharya, C.; Bhattacharya, S.; Bhattacharyya, S.; Gehlot, J.; Ghugre, S. S.; Gurjar, R. K.; Jhingan, A.; Kumar, R.; Muralithar, S.; Nath, S.; Pai, H.; Palit, R.; Raut, R.; Singh, R. P.; Sinha, A. K.; Varughese, T.

    2015-11-01

    A new high-spin isomer has been identified in 195Bi at the focal plane of the HYbrid Recoil mass Analyser (HYRA) used in the gas-filled mode. The fusion evaporation reactions 169Tm (30Si, x n) 193, 195Bi were used with the beam energies on targets of 168 and 146MeV for 6n and 4n channels, respectively. The evaporation residues, separated from the fission fragments, and their decays were detected at the focal plane of HYRA using MWPC, Si-Pad and clover HPGe detectors. The half-life of the new isomer in 195Bi has been measured to be 1.6(1)μs. The configuration of the new isomer has been proposed and compared with the other isomers in this region. The Total Routhian Surface (TRS) calculations for the three-quasiparticle configurations corresponding to the new isomer suggest an oblate deformation for this isomeric state. The same calculations for different configurations in 195Bi and for the even-even 194Pb core indicate that the proton i 13/2 orbital has a large shape driving effect towards oblate shape in these nuclei.

  12. Competition between collective and noncollective excitation modes at high spin in Ba124

    NASA Astrophysics Data System (ADS)

    Al-Khatib, A.; Singh, A. K.; Hübel, H.; Bringel, P.; Bürger, A.; Domscheit, J.; Neußer-Neffgen, A.; Schönwaßer, G.; Hagemann, G. B.; Hansen, C. Ronn; Herskind, B.; Sletten, G.; Wilson, J. N.; Timár, J.; Algora, A.; Dombrádi, Zs.; Gál, J.; Kalinka, G.; Molnár, J.; Nyakó, B. M.; Sohler, D.; Zolnai, L.; Clark, R. M.; Cromaz, M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Ward, D.; Amro, H.; Ma, W. C.; Kmiecik, M.; Maj, A.; Styczen, J.; Zuber, K.; Hauschild, K.; Korichi, A.; Lopez-Martens, A.; Roccaz, J.; Siem, S.; Hannachi, F.; Scheurer, J. N.; Bednarczyk, P.; Byrski, Th.; Curien, D.; Dorvaux, O.; Duchêne, G.; Gall, B.; Khalfallah, F.; Piqueras, I.; Robin, J.; Görgen, A.; Juhász, K.; Patel, S. B.; Evans, A. O.; Rainovski, G.; Benzoni, G.; Bracco, A.; Camera, F.; Leoni, S.; Mason, P.; Million, B.; Paleni, A.; Sacchi, R.; Wieland, O.; Petrache, C. M.; Petrache, D.; Rana, G. La; Moro, R.; De Angelis, G.; Lisle, J. C.; Cederwall, B.; Lagergren, K.; Lieder, R. M.; Podsvirova, E.; Gast, W.; Jäger, H.; Redon, N.

    2006-07-01

    High-spin states in Ba124 were investigated in two experiments using the Ni64(Ni64, 4n)Ba124 reaction at three different beam energies. In-beam γ-ray coincidences were measured with the Euroball and Gammasphere detector arrays. In the experiment with Euroball, the CsI detector array Diamant was employed to discriminate against charged-particle channels. Six new rotational bands were observed in Ba124, and previously known bands were extended to higher spins. One of the bands shows a transition from collective to noncollective behavior at high spins. Configuration assignments are suggested on the basis of comparison with cranked shell model and cranked Nilsson-Strutinsky calculations.

  13. Observation of high-spin oblate band structures in {sup 141}Pm

    SciTech Connect

    Gu, L.; Zhu, S. J.; Wang, J. G.; Yeoh, E. Y.; Xiao, Z. G.; Zhang, M.; Liu, Y.; Ding, H. B.; Xu, Q.; Zhang, S. Q.; Meng, J.; Zhu, L. H.; Wu, X. G.; He, C. Y.; Li, G. S.; Wang, L. L.; Zheng, Y.; Zhang, B.

    2011-06-15

    The high-spin states of {sup 141}Pm have been investigated through the reaction {sup 126}Te({sup 19}F,4n) at a beam energy of 90 MeV. A previous level scheme has been updated with spins up to 49/2({h_bar}/2{pi}). Six collective bands at high spins are newly observed. Based on the systematic comparison, one band is proposed as a decoupled band; two bands with strong {Delta}I=1 M1 transitions inside the bands are suggested as the oblate bands with {gamma} {approx}-60 deg.; three other bands with large signature splitting have been proposed with the oblate-triaxial deformation with {gamma}{approx} -90 deg. The triaxial n-particle-n-hole particle rotor model calculations for one of the oblate bands in {sup 141}Pm are in good agreement with the experimental data. The other characteristics for these bands have been discussed.

  14. High Efficiency Spin Flipper for the n3He Experiment

    NASA Astrophysics Data System (ADS)

    Hayes, Christopher; n3He Collaboration

    2015-10-01

    The n3He experiment, constructed on the Fundamental Neutron Physics Beamline (FnPB) at the Spallation Neutron Source, is designed to measure the parity violating (PV) proton asymmetry Ap in the capture reaction n +3 He -->3 H + p + 765 keV The asymmetry has an estimated value Ap ~ - 1 ×10-7 and is directly related to the weak isospin conserved couplings hρ0 and ωρ0 which are of fundamental interest in the verification of the meson exchange model of low energy NN intereactions. Data production for the n3He experiment began in February 2015 and is scheduled to continue thru December 2015 - reaching a statistical sensitivity δAp ~10-8 or better. I will discuss the spin flipper which is designed using the theory of double cosine-theta coils, and capable of flipping neutron spins with an efficiency approaching its maximum value ɛsf = 1 . I will also discuss the theory of Spin Magnetic Resonance (SMR) and how it is employed by the spin flipper to flip 60 Hz pulses of cold neutrons over a range of wavelengths.

  15. Observing bulk diamond spin coherence in high-purity nanodiamonds.

    PubMed

    Knowles, Helena S; Kara, Dhiren M; Atatüre, Mete

    2014-01-01

    Nitrogen-vacancy (NV) centres in diamond are attractive for research straddling quantum information science, nanoscale magnetometry and thermometry. Whereas ultrapure bulk diamond NVs sustain the longest spin coherence times among optically accessible spins, nanodiamond NVs exhibit persistently poor spin coherence. Here we introduce high-purity nanodiamonds accommodating record-long NV coherence times, >60 μs, observed through universal dynamical decoupling. We show that the main contribution to decoherence comes from nearby nitrogen impurities rather than surface states. We protect the NV spin free precession, essential to d.c. magnetometry, by driving solely these impurities into the motional narrowing regime. This extends the NV free induction decay time from 440 ns, longer than that in type Ib bulk diamond, to 1.27 μs, which is comparable to that in type IIa (impurity-free) diamond. These properties allow the simultaneous exploitation of both high sensitivity and nanometre resolution in diamond-based emergent quantum technologies. PMID:24270582

  16. High-Spin Organic Diradical with Robust Stability.

    PubMed

    Gallagher, Nolan M; Bauer, Jackson J; Pink, Maren; Rajca, Suchada; Rajca, Andrzej

    2016-08-01

    Triplet ground-state organic molecules are interesting with respect to several emerging technologies but typically exhibit limited stability. We report two organic diradicals, one of which possesses a triplet ground state (2J/kB = 234 ± 36 K) and robust stability at elevated temperatures. We are able to sublime this high-spin diradical under high vacuum at 140 °C with no significant decomposition. PMID:27430499

  17. Collective mode evidence of high-spin bosonization in a trapped one-dimensional atomic Fermi gas with tunable spin

    SciTech Connect

    Liu, Xia-Ji Hu, Hui

    2014-11-15

    We calculate the frequency of collective modes of a one-dimensional repulsively interacting Fermi gas with high-spin symmetry confined in harmonic traps at zero temperature. This is a system realizable with fermionic alkaline-earth-metal atoms such as {sup 173}Yb, which displays an exact SU(κ) spin symmetry with κ⩾2 and behaves like a spinless interacting Bose gas in the limit of infinite spin components κ→∞, namely high-spin bosonization. We solve the homogeneous equation of state of the high-spin Fermi system by using Bethe ansatz technique and obtain the density distribution in harmonic traps based on local density approximation. The frequency of collective modes is calculated by exactly solving the zero-temperature hydrodynamic equation. In the limit of large number of spin-components, we show that the mode frequency of the system approaches that of a one-dimensional spinless interacting Bose gas, as a result of high-spin bosonization. Our prediction of collective modes is in excellent agreement with a very recent measurement for a Fermi gas of {sup 173}Yb atoms with tunable spin confined in a two-dimensional tight optical lattice.

  18. Nanoscale Magnetic Materials for Energy-Efficient Spin Based Transistors

    NASA Astrophysics Data System (ADS)

    Incorvia, Jean Anne Currivan

    In this dissertation, I study the physical behavior of nanoscale magnetic materials and build spin-based transistors that encode information in magnetic domain walls. It can be argued that energy dissipation is the most serious problem in modern electronics, and one that has been resistant to a breakthrough. Wasted heat during computing both wastes energy and hinders further technology scaling. This is an opportunity for physicists and engineers to come up with creative solutions for more energy-efficient computing. I present the device we have designed, called domain wall logic (DW-Logic). Information is stored in the position of a magnetic domain wall in a ferromagnetic wire and read out using a magnetic tunnel junction. This hybrid design uses electrical current as the input and output, keeping the device compatible with charge- based transistors. I build an iterative model to predict both the micromagnetic and circuit behavior of DW- Logic, showing a single device can operate as a universal gate. The model shows we can build complex circuits including an 18-gate Full Adder, and allows us to predict the device switching energy compared to complementary metal-oxide semiconductor (CMOS) transistors. Comparing ?15 nm feature nodes, I find DW-Logic made with perpendicular magnetic anisotropy materials, and utilizing both spin torque transfer and the Spin Hall effect, could operate with 1000x reduced switching energy compared to CMOS. I fabricate DW-Logic device prototypes and show in experiment they can act as AND and NAND gates. I demonstrate that one device can drive two subsequent devices, showing gain, which is a necessary requirement for fanout. I also build a clocked ring oscillator circuit to demonstrate successful bit propagation in a DW-Logic circuit and show that properly scaled devices can have improved operation. Through building the devices, I develop a novel fabrication method for patterning sub-25 nm magnetic wires with very low (˜ 2 nm) average edge

  19. High-spin. gamma. -ray spectroscopy: past successes, future hopes

    SciTech Connect

    Diamond, R.M.

    1983-04-01

    Nuclei can carry angular momentum by aligning individual particles along the rotation axis or by rotation of a deformed nucleus as a whole. The interweaving of these modes leads to a variety of behavior that is just beginning to be observed and explained. The discrete ..gamma..-ray studies have led to a new backbending spectroscopy, which is telling us about the details of particle alignments and monopole and quadrupole pairing. The high-spin continuum studies, as yet less well developed, are indicating changes in shape and structure, as well as particle alignments from higher shells. New developments in detector systems and in theory promise much more detailed comparisons of experiment and theory and consequent increase in our knowledge of nuclear behavior at high spin.

  20. High-spin nuclear structure data on the Internet

    SciTech Connect

    Singh, B. |

    1997-12-31

    The study of nuclear structure at fast nuclear rotations, using fusion-evaporation reactions, started in the early sixties but since the experimental observation of superdeformation about a decade ago it has become one of the most pursued research topics in nuclear physics. Large gamma-ray detector arrays GAMMASPHERE, EUROGAM, and GASP were developed during the last few years and these continue to produce a wealth of new, information about the properties of nuclei at high spins, including superdeformation. It is considered vital to compile, evaluate and systematize published data on many thousands of levels and gamma rays and associated nuclear bands obtained in such studies and make these available to the research community in conveniently retrievable and modern formats. This talk will describe the numerical, bibliographic and other high-spin related databases that are already accessible via INTERNET. Present limitations and ways to improve the current status and display of such databases will also be discussed.

  1. Lifetime measurement of high spin states in (75) Kr

    SciTech Connect

    Sheikh, Javid; Trivedi, T.; Maurya, K.; Mehrotra, I.; Palit, R.; Naik, Z.; Jain, H. C.; Negi, D.; Mahanto, G.; Kumar, R.; Singh, R.P.; Muralithar, S.; Pancholi, S.C.; Bhowmik, R.K.; Yang, Y-C; Sun, Y.; Dahl, A.; Raju, M.K.; Appannababu, S.; Kumar, S.; Choudhury, D.; Jain, A. K.

    2010-01-01

    The lifetimes of high spin states of {sup 75}Kr have been determined via {sup 50}Cr ({sup 28}Si, 2pn) {sup 75}Kr reaction in positive parity band using the Doppler-shift attenuation method. The transition quadrupole moments Q deduced from lifetime measurements have been compared with {sup 75}Br. Experimental results obtained from lifetime measurement are interpreted in the framework of projected shell model.

  2. High-mobility ultrathin semiconducting films prepared by spin coating

    NASA Astrophysics Data System (ADS)

    Mitzi, David B.; Kosbar, Laura L.; Murray, Conal E.; Copel, Matthew; Afzali, Ali

    2004-03-01

    The ability to deposit and tailor reliable semiconducting films (with a particular recent emphasis on ultrathin systems) is indispensable for contemporary solid-state electronics. The search for thin-film semiconductors that provide simultaneously high carrier mobility and convenient solution-based deposition is also an important research direction, with the resulting expectations of new technologies (such as flexible or wearable computers, large-area high-resolution displays and electronic paper) and lower-cost device fabrication. Here we demonstrate a technique for spin coating ultrathin (~50Å), crystalline and continuous metal chalcogenide films, based on the low-temperature decomposition of highly soluble hydrazinium precursors. We fabricate thin-film field-effect transistors (TFTs) based on semiconducting SnS2-xSex films, which exhibit n-type transport, large current densities (>105Acm-2) and mobilities greater than 10cm2V-1s-1-an order of magnitude higher than previously reported values for spin-coated semiconductors. The spin-coating technique is expected to be applicable to a range of metal chalcogenides, particularly those based on main group metals, as well as for the fabrication of a variety of thin-film-based devices (for example, solar cells, thermoelectrics and memory devices).

  3. Orientation estimation algorithm applied to high-spin projectiles

    NASA Astrophysics Data System (ADS)

    Long, D. F.; Lin, J.; Zhang, X. M.; Li, J.

    2014-06-01

    High-spin projectiles are low cost military weapons. Accurate orientation information is critical to the performance of the high-spin projectiles control system. However, orientation estimators have not been well translated from flight vehicles since they are too expensive, lack launch robustness, do not fit within the allotted space, or are too application specific. This paper presents an orientation estimation algorithm specific for these projectiles. The orientation estimator uses an integrated filter to combine feedback from a three-axis magnetometer, two single-axis gyros and a GPS receiver. As a new feature of this algorithm, the magnetometer feedback estimates roll angular rate of projectile. The algorithm also incorporates online sensor error parameter estimation performed simultaneously with the projectile attitude estimation. The second part of the paper deals with the verification of the proposed orientation algorithm through numerical simulation and experimental tests. Simulations and experiments demonstrate that the orientation estimator can effectively estimate the attitude of high-spin projectiles. Moreover, online sensor calibration significantly enhances the estimation performance of the algorithm.

  4. Magnetic field induced spin-wave energy focusing

    NASA Astrophysics Data System (ADS)

    Perez, Noel; Lopez-Diaz, Luis

    2015-07-01

    Local temperature variations induced by spin-wave propagation are studied using a model that couples nonuniform magnetization dynamics and heat flow. We show that the remote heating at the sample edge reported recently [T. An et al., Nat. Mater. 12, 549 (2013)], 10.1038/nmat3628 is due to the geometry-induced gradual reduction of the effective field. We demonstrate that the same effect can be achieved by a reduction in the external field instead of a constriction at the edge and, furthermore, that both the location and the amount of energy to be delivered to the lattice can be controlled accurately this way.

  5. Possible enhancements of AFM spin-fluctuations in high-TC cuprates

    NASA Astrophysics Data System (ADS)

    Jarlborg, Thomas

    2009-03-01

    Ab-initio band calculations for high-TC cuprates, together with modelling based of a free electron like band, show a strong interaction between anti-ferromagnetic (AFM) spin waves and periodic lattice distortions as for phonons, even though this type of spin-phonon coupling (SPC) is underestimated in calculations using the local density approximation. The SPC has a direct influence on the properties of the HTC cuprates and it can explain many observations. The strongest effects are seen for modulated waves in the CuO bond direction, and a band gap is formed near the X,Y points, but unusal band dispersion (like ``waterfalls'') might also be induced below the Fermi energy (EF) in the diagonal direction. The band results are used to propose different ways of increasing AFM spin-fluctuations locally, and to have a higher density-of-states (DOS) at EF. Static potential modulations, via periodic distribution of dopants or lattice distortions, can be tuned to increase the DOS. This opens for possibilities to enhance coupling for spin fluctuations (λsf) and superconductivity. The exchange enhancement is in general increased near a surface, which suggests a tendency towards static spin configurations. The sensivity of the band results to corrections of the local density potential are discussed.

  6. Competing decay modes of a high-spin isomer in the proton-unbound nucleus ¹⁵⁸Ta*

    DOE PAGESBeta

    Carroll, R. J.; Page, R. D.; Joss, D. T.; Uusitalo, J.; Darby, I. G.; Andgren, K.; Cederwall, B.; Eeckhaudt, S.; Grahn, T.; Gray-Jones, C.; et al

    2015-01-01

    An isomeric state at high spin and excitation energy was recently observed in the proton-unbound nucleus 158Ta. This state was observed to decay by both α and γ decay modes. The large spin change required to decay via γ-ray emission incurs a lifetime long enough for α decay to compete. The α decay has an energy of 8644(11) keV, which is among the highest observed in the region, a partial half-life of 440(70) μs and changes the spin by 11ℏ. In this study, additional evidence supporting the assignment of this α decay to the high-spin isomer in 158Ta will bemore » presented.« less

  7. Competing decay modes of a high-spin isomer in the proton-unbound nucleus ¹⁵⁸Ta*

    SciTech Connect

    Carroll, R. J.; Page, R. D.; Joss, D. T.; Uusitalo, J.; Darby, I. G.; Andgren, K.; Cederwall, B.; Eeckhaudt, S.; Grahn, T.; Gray-Jones, C.; Greenlees, P. T.; Hadinia, B.; Jones, P. M.; Julin, R.; Juutinen, S.; Leino, M.; Leppänen, A. -P.; Nyman, M.; O'Donnell, D.; Pakarinen, J.; Rahkila, P.; Sandzelius, M.; Sarén, J.; Scholey, C.; Seweryniak, D.; Simpson, J.

    2015-01-01

    An isomeric state at high spin and excitation energy was recently observed in the proton-unbound nucleus 158Ta. This state was observed to decay by both α and γ decay modes. The large spin change required to decay via γ-ray emission incurs a lifetime long enough for α decay to compete. The α decay has an energy of 8644(11) keV, which is among the highest observed in the region, a partial half-life of 440(70) μs and changes the spin by 11ℏ. In this study, additional evidence supporting the assignment of this α decay to the high-spin isomer in 158Ta will be presented.

  8. Collectivity of high spin states in {sup 84}Zr

    SciTech Connect

    Lister, C.J.; Blumenthal, D.; Crowell, B.

    1995-08-01

    {sup 84}Zr is one of the most extensively studied of the A {approximately} 80 rotors, both from theoretical and experimental approaches. It was predicted to be a good candidate to support superdeformation, and to show interesting spectroscopic properties including saturation of its shell-model space at lower spin. We performed an experiment using Gammasphere in its early implementation phase. The reaction of {sup 29}Si on {sup 58}Ni was used to strongly populate {sup 84}Zr at high spin. Thin and thick targets were used to allow the extraction of transitional matrix elements at very high spin, and to allow a sensitive search for superdeformed states. Data analysis is in progress. The large data set allowed us to extend the previously known bands considerably. Candidates for a staggered M1-band, found previously {sup 86}Zr, were located. To date, no evidence for superdeformed bands was found. Analysis was slowed by the relocation of all the participants in this experiment, but we hope to complete the lifetime analysis this year. This analysis has become especially topical, due to reported measurements of superdeformation in this region.

  9. Equation-of-motion coupled cluster method for high spin double electron attachment calculations

    SciTech Connect

    Musiał, Monika Lupa, Łukasz; Kucharski, Stanisław A.

    2014-03-21

    The new formulation of the equation-of-motion (EOM) coupled cluster (CC) approach applicable to the calculations of the double electron attachment (DEA) states for the high spin components is proposed. The new EOM equations are derived for the high spin triplet and quintet states. In both cases the new equations are easier to solve but the substantial simplification is observed in the case of quintets. Out of 21 diagrammatic terms contributing to the standard DEA-EOM-CCSDT equations for the R{sub 2} and R{sub 3} amplitudes only four terms survive contributing to the R{sub 3} part. The implemented method has been applied to the calculations of the excited states (singlets, triplets, and quintets) energies of the carbon and silicon atoms and potential energy curves for selected states of the Na{sub 2} (triplets) and B{sub 2} (quintets) molecules.

  10. High Frequency QPOs due to Black Hole Spin

    NASA Technical Reports Server (NTRS)

    Kazanas, Demos; Fukumura, K.

    2009-01-01

    We present detailed computations of photon orbits emitted by flares at the innermost stable circular orbit (ISCO) of accretion disks around rotating black holes. We show that for sufficiently large spin parameter, i.e. a > 0.94 M, flare a sufficient number of photons arrive at an observer after multiple orbits around the black hole, to produce an "photon echo" of constant lag, i.e. independent of the relative phase between the black hole and the observer, of T approximates 14 M. This constant time delay, then, leads to a power spectrum with a QPO at a frequency nu approximates 1/14M, even for a totally random ensemble of such flares. Observation of such a QPO will provide incontrovertible evidence for the high spin of the black hole and a very accurate, independent, measurement of its mass.

  11. A high-efficiency spin-resolved photoemission spectrometer combining time-of-flight spectroscopy with exchange-scattering polarimetry

    SciTech Connect

    Jozwiak, Chris M.; Graff, Jeff; Lebedev, Gennadi; Andresen, Nord; Schmid, Andreas; Fedorov, Alexei; El Gabaly, Farid; Wan, Weishi; Lanzara, Alessandra; Hussain, Zahid

    2010-04-13

    We describe a spin-resolved electron spectrometer capable of uniquely efficient and high energy resolution measurements. Spin analysis is obtained through polarimetry based on low-energy exchange scattering from a ferromagnetic thin-film target. This approach can achieve a similar analyzing power (Sherman function) as state-of-the-art Mott scattering polarimeters, but with as much as 100 times improved efficiency due to increased reflectivity. Performance is further enhanced by integrating the polarimeter into a time-of-flight (TOF) based energy analysis scheme with a precise and flexible electrostatic lens system. The parallel acquisition of a range of electron kinetic energies afforded by the TOF approach results in an order of magnitude (or more) increase in efficiency compared to hemispherical analyzers. The lens system additionally features a 90 degrees bandpass filter, which by removing unwanted parts of the photoelectron distribution allows the TOF technique to be performed at low electron drift energy and high energy resolution within a wide range of experimental parameters. The spectrometer is ideally suited for high-resolution spin- and angle-resolved photoemission spectroscopy (spin-ARPES), and initial results are shown. The TOF approach makes the spectrometer especially ideal for time-resolved spin-ARPES experiments.

  12. High energy neutron radiography

    SciTech Connect

    Gavron, A.; Morley, K.; Morris, C.; Seestrom, S.; Ullmann, J.; Yates, G.; Zumbro, J.

    1996-06-01

    High-energy spallation neutron sources are now being considered in the US and elsewhere as a replacement for neutron beams produced by reactors. High-energy and high intensity neutron beams, produced by unmoderated spallation sources, open potential new vistas of neutron radiography. The authors discuss the basic advantages and disadvantages of high-energy neutron radiography, and consider some experimental results obtained at the Weapons Neutron Research (WNR) facility at Los Alamos.

  13. High frequency spin torque oscillators with composite free layer spin valve

    NASA Astrophysics Data System (ADS)

    Natarajan, Kanimozhi; Arumugam, Brinda; Rajamani, Amuda

    2016-07-01

    We report the oscillations of magnetic spin components in a composite free layer spin valve. The associated Landau-Lifshitz-Gilbert-Slonczewski (LLGS) equation is studied by stereographically projecting the spin on to a complex plane and the spin components were found. A fourth order Runge-Kutta numerical integration on LLGS equation also confirms the similar trajectories of the spin components. This study establishes the possibility of a Spin Torque Oscillator in a composite free layer spin valve, where the exchange coupling is ferromagnetic in nature. In-plane and out-of-plane precessional modes of magnetization oscillations were found in zero applied magnetic field and the frequencies of the oscillations were calculated from Fast Fourier Transform of the components of magnetization. Behavior of Power Spectral Density for a range of current density is studied. Finally our analysis shows the occurrence of highest frequency 150 GHz, which is in the second harmonics for the specific choice of system parameters.

  14. High-resolution three-dimensional spin- and angle-resolved photoelectron spectrometer using vacuum ultraviolet laser light

    NASA Astrophysics Data System (ADS)

    Yaji, Koichiro; Harasawa, Ayumi; Kuroda, Kenta; Toyohisa, Sogen; Nakayama, Mitsuhiro; Ishida, Yukiaki; Fukushima, Akiko; Watanabe, Shuntaro; Chen, Chuangtian; Komori, Fumio; Shin, Shik

    2016-05-01

    We describe a spin- and angle-resolved photoelectron spectroscopy (SARPES) apparatus with a vacuum-ultraviolet (VUV) laser (hν = 6.994 eV) developed at the Laser and Synchrotron Research Center at the Institute for Solid State Physics, The University of Tokyo. The spectrometer consists of a hemispherical photoelectron analyzer equipped with an electron deflector function and twin very-low-energy-electron-diffraction-type spin detectors, which allows us to analyze the spin vector of a photoelectron three-dimensionally with both high energy and angular resolutions. The combination of the high-performance spectrometer and the high-photon-flux VUV laser can achieve an energy resolution of 1.7 meV for SARPES. We demonstrate that the present laser-SARPES machine realizes a quick SARPES on the spin-split band structure of a Bi(111) film even with 7 meV energy and 0.7∘ angular resolutions along the entrance-slit direction. This laser-SARPES machine is applicable to the investigation of spin-dependent electronic states on an energy scale of a few meV.

  15. High-resolution three-dimensional spin- and angle-resolved photoelectron spectrometer using vacuum ultraviolet laser light.

    PubMed

    Yaji, Koichiro; Harasawa, Ayumi; Kuroda, Kenta; Toyohisa, Sogen; Nakayama, Mitsuhiro; Ishida, Yukiaki; Fukushima, Akiko; Watanabe, Shuntaro; Chen, Chuangtian; Komori, Fumio; Shin, Shik

    2016-05-01

    We describe a spin- and angle-resolved photoelectron spectroscopy (SARPES) apparatus with a vacuum-ultraviolet (VUV) laser (hν = 6.994 eV) developed at the Laser and Synchrotron Research Center at the Institute for Solid State Physics, The University of Tokyo. The spectrometer consists of a hemispherical photoelectron analyzer equipped with an electron deflector function and twin very-low-energy-electron-diffraction-type spin detectors, which allows us to analyze the spin vector of a photoelectron three-dimensionally with both high energy and angular resolutions. The combination of the high-performance spectrometer and the high-photon-flux VUV laser can achieve an energy resolution of 1.7 meV for SARPES. We demonstrate that the present laser-SARPES machine realizes a quick SARPES on the spin-split band structure of a Bi(111) film even with 7 meV energy and 0.7(∘) angular resolutions along the entrance-slit direction. This laser-SARPES machine is applicable to the investigation of spin-dependent electronic states on an energy scale of a few meV. PMID:27250396

  16. Electron spin density on the axial His ligand of high-spin and low-spin Nitrophorin 2 probed by heteronuclear NMR spectroscopy

    PubMed Central

    Abriata, Luciano A.; Zaballa, María-Eugenia; Berry, Robert E.; Yang, Fei; Zhang, Hongjun; Walker, F. Ann; Vila, Alejandro J.

    2013-01-01

    The electronic structure of heme proteins is exquisitely tuned by the interaction of the iron center with the axial ligands. NMR studies of paramagnetic heme systems have been focused on the heme signals, but signals from the axial ligands have been rather difficult to detect and assign. We report an extensive assignment of the 1H, 13C and 15N resonances of the axial His ligand in the NO-carrying protein nitrophorin 2 (NP2) in the paramagnetic high-spin and low-spin forms, as well as in the diamagnetic NO complex. We find that the high-spin protein has σ spin delocalization to all atoms in the axial His57, which decreases in size as the number of bonds between Fe(III) and the atom in question increase, except that within the His57 imidazole ring the contact shifts are a balance between positive σ and negative π contributions. In contrast, the low-spin protein has π spin delocalization to all atoms of the imidazole ring. Our strategy, adequately combined with a selective residue labeling scheme, represents a straightforward characterization of the electron spin density in heme axial ligands. PMID:23327568

  17. Efficient rotational echo double resonance recoupling of a spin-1/2 and a quadrupolar spin at high spinning rates and weak irradiation fields

    NASA Astrophysics Data System (ADS)

    Nimerovsky, Evgeny; Goldbourt, Amir

    2010-09-01

    A modification of the rotational echo (adiabatic passage) double resonance experiments, which allows recoupling of the dipolar interaction between a spin-1/2 and a half integer quadrupolar spin is proposed. We demonstrate efficient and uniform recoupling at high spinning rates ( ν r), low radio-frequency (RF) irradiation fields ( ν1), and high values of the quadrupolar interaction ( ν q) that correspond to values of α=ν12/νqνr, the adiabaticity parameter, which are down to less than 10% of the traditional adiabaticity limit for a spin-5/2 (α = 0.55). The low-alpha rotational echo double resonance curve is obtained when the pulse on the quadrupolar nucleus is extended to full two rotor periods and beyond. For protons (spin-1/2) and aluminum (spin-5/2) species in the zeolite SAPO-42, a dephasing curve, which is significantly better than the regular REAPDOR experiment (pulse length of one-third of the rotor period) is obtained for a spinning rate of 13 kHz and RF fields down to 10 and even 6 kHz. Under these conditions, α is estimated to be approximately 0.05 based on an average quadrupolar coupling in zeolites. Extensive simulations support our observations suggesting the method to be robust under a large range of experimental values.

  18. High-spin torus isomers and their precession motions

    NASA Astrophysics Data System (ADS)

    Ichikawa, T.; Matsuyanagi, K.; Maruhn, J. A.; Itagaki, N.

    2014-09-01

    Background: In our previous study, we found that an exotic isomer with a torus shape may exist in the high-spin, highly excited states of Ca40. The z component of the total angular momentum, Jz=60ℏ, of this torus isomer is constructed by totally aligning 12 single-particle angular momenta in the direction of the symmetry axis of the density distribution. The torus isomer executes precession motion with the rigid-body moments of inertia about an axis perpendicular to the symmetry axis. The investigation, however, has been focused only on Ca40. Purpose: We systematically investigate the existence of exotic torus isomers and their precession motions for a series of N =Z even-even nuclei from Si28 to Ni56. We analyze the microscopic shell structure of the torus isomer and discuss why the torus shape is generated beyond the limit of large oblate deformation. Method: We use the cranked three-dimensional Hartree-Fock method with various Skyrme interactions in a systematic search for high-spin torus isomers. We use the three-dimensional time-dependent Hartree-Fock method for describing the precession motion of the torus isomer. Results: We obtain high-spin torus isomers in Ar36,Ca40,Ti44,Cr48, and Fe52. The emergence of the torus isomers is associated with the alignments of single-particle angular momenta, which is the same mechanism as found in Ca40. It is found that all the obtained torus isomers execute the precession motion at least two rotational periods. The moment of inertia about a perpendicular axis, which characterizes the precession motion, is found to be close to the classical rigid-body value. Conclusions: The high-spin torus isomer of Ca40 is not an exceptional case. Similar torus isomers exist widely in nuclei from Ar36 to Fe52 and they execute the precession motion. The torus shape is generated beyond the limit of large oblate deformation by eliminating the 0s components from all the deformed single-particle wave functions to maximize their mutual

  19. Spin transport at high temperatures in epitaxial Heusler alloy/n-GaAs lateral spin valves

    NASA Astrophysics Data System (ADS)

    Peterson, Timothy A.; Christie, Kevin D.; Patel, Sahil J.; Crowell, Paul A.; Palmstrøm, Chris J.

    2015-03-01

    We report on electrical injection and detection of spin accumulation in ferromagnet/ n-GaAs lateral spin-valve devices, observed up to and above room temperature. The ferromagnet in these measurements is the Heusler alloy Co2FeSi, and the semiconductor channel is GaAs doped at 3 ×1016 cm-3. The spin signal is enhanced by operating the detection contact under forward bias. The enhancement originates from drift effects at low-temperatures and an increase of the detection efficiency at all temperatures. The detector bias dependence of the observed spin-valve signal is interpreted by taking into account the quantum well (QW) which forms in the degenerately doped region immediately behind the Schottky tunnel barrier. In particular, we believe the QW is responsible for the minority spin accumulation (majority spin current) under large forward bias. The spin diffusion length and lifetime are determined by measuring the separation dependence of the non-local spin valve signal in a family of devices patterned by electron beam lithography. A spin diffusion length of 700 nm and lifetime of 46 picoseconds are found at a temperature of 295 K. This work was supported by the NSF under DMR-1104951, the NSF MRSEC program and C-SPIN, a SRC STARNET center sponsored by MARCO and DARPA.

  20. Spin dynamics in relativistic ionization with highly charged ions in super-strong laser fields

    NASA Astrophysics Data System (ADS)

    Klaiber, Michael; Yakaboylu, Enderalp; Müller, Carsten; Bauke, Heiko; Paulus, Gerhard G.; Hatsagortsyan, Karen Z.

    2014-03-01

    Spin dynamics and induced spin effects in above-threshold ionization of hydrogenlike highly charged ions in super-strong laser fields are investigated. Spin-resolved ionization rates in the tunnelling regime are calculated by employing two versions of a relativistic Coulomb-corrected strong-field approximation (SFA). An intuitive simpleman model is developed which explains the derived scaling laws for spin flip and spin asymmetry effects. The intuitive model as well as our ab initio numerical simulations support the analytical results for the spin effects obtained in the dressed SFA where the impact of the laser field on the electron spin evolution in the bound state is taken into account. In contrast, the standard SFA is shown to fail in reproducing spin effects in ionization even at a qualitative level. The anticipated spin-effects are expected to be measurable with modern laser techniques combined with an ion storage facility.

  1. Complete High-Spin Structure of 57Co

    SciTech Connect

    Caballero, O. L.; Christancho, F.; Rudolph, D.; Baktash, Cyrus; Devlin, M.; Riedinger, Lee L; Sarantites, D. G.; Yu, Chang-Hong

    2003-02-01

    A comprehensive high-spin decay scheme has been deduced for {sup 57}Co using the Gammasphere Germanium detector array coupled to the 4{pi} charged-particle detector system Microball. Following the fusion-evaporation reaction of {sup 28}Si({sup 36}Ar,1{alpha}3p){sup 57}Co at 136 MeV beam energy about 90 excited states have been observed in {sup 57}Co, which are connected by some 230 {gamma}-ray transitions. The proposed level scheme reaches 16 MeV excitation energy at a spin of 17{Dirac_h} 18{Dirac_h}. With its complexity the level scheme of {sup 57}Co appears to be 'complete' up to 1 or 2 MeV above the yrast line. This aspect is further investigated through a comparison of the data with spherical shell-model calculations.

  2. Ground-state energies of the nonlinear sigma model and the Heisenberg spin chains

    NASA Technical Reports Server (NTRS)

    Zhang, Shoucheng; Schulz, H. J.; Ziman, Timothy

    1989-01-01

    A theorem on the O(3) nonlinear sigma model with the topological theta term is proved, which states that the ground-state energy at theta = pi is always higher than the ground-state energy at theta = 0, for the same value of the coupling constant g. Provided that the nonlinear sigma model gives the correct description for the Heisenberg spin chains in the large-s limit, this theorem makes a definite prediction relating the ground-state energies of the half-integer and the integer spin chains. The ground-state energies obtained from the exact Bethe ansatz solution for the spin-1/2 chain and the numerical diagonalization on the spin-1, spin-3/2, and spin-2 chains support this prediction.

  3. A 3D-printed high power nuclear spin polarizer.

    PubMed

    Nikolaou, Panayiotis; Coffey, Aaron M; Walkup, Laura L; Gust, Brogan M; LaPierre, Cristen D; Koehnemann, Edward; Barlow, Michael J; Rosen, Matthew S; Goodson, Boyd M; Chekmenev, Eduard Y

    2014-01-29

    Three-dimensional printing with high-temperature plastic is used to enable spin exchange optical pumping (SEOP) and hyperpolarization of xenon-129 gas. The use of 3D printed structures increases the simplicity of integration of the following key components with a variable temperature SEOP probe: (i) in situ NMR circuit operating at 84 kHz (Larmor frequencies of (129)Xe and (1)H nuclear spins), (ii) <0.3 nm narrowed 200 W laser source, (iii) in situ high-resolution near-IR spectroscopy, (iv) thermoelectric temperature control, (v) retroreflection optics, and (vi) optomechanical alignment system. The rapid prototyping endowed by 3D printing dramatically reduces production time and expenses while allowing reproducibility and integration of "off-the-shelf" components and enables the concept of printing on demand. The utility of this SEOP setup is demonstrated here to obtain near-unity (129)Xe polarization values in a 0.5 L optical pumping cell, including ∼74 ± 7% at 1000 Torr xenon partial pressure, a record value at such high Xe density. Values for the (129)Xe polarization exponential build-up rate [(3.63 ± 0.15) × 10(-2) min(-1)] and in-cell (129)Xe spin-lattice relaxation time (T1 = 2.19 ± 0.06 h) for 1000 Torr Xe were in excellent agreement with the ratio of the gas-phase polarizations for (129)Xe and Rb (PRb ∼ 96%). Hyperpolarization-enhanced (129)Xe gas imaging was demonstrated with a spherical phantom following automated gas transfer from the polarizer. Taken together, these results support the development of a wide range of chemical, biochemical, material science, and biomedical applications. PMID:24400919

  4. Magnetic anisotropy and high-spin effects in single-molecule transistors

    NASA Astrophysics Data System (ADS)

    Zyazin, Alexander; van den Berg, Johan; Osorio, Edgar; Konstantinidis, Nikos; Leijnse, Martin; May, Falk; Hofstetter, Walter; Danieli, Chiara; Cornia, Andrea; Wegewijs, Maarten; van der Zant, Herre

    2011-03-01

    Fabrication of single-molecule transistors where electron transport occurs through an individual molecule has become possible due to the recent progress in molecular electronics. Three-terminal configuration allows charging molecules and performing transport spectroscopy in multiple redox states. Single-molecule magnets combining large spin with uniaxial anisotropy are of special interest as appealing candidates for high density memory applications and quantum information processing. We study single-molecule magnets Fe 4 . Three-terminal junctions are fabricated using electromigration of gold nanowires followed by a self-breaking. High-spin Kondo effect and inelastic cotunneling excitations show up in transport measurements. Several excitations feature the energy close to the energy of zero-field splitting (ZFS) of a ground spin multiplet in bulk. This splitting is caused by the anisotropy and is a hallmark of single-molecule magnets. We observe nonlinear Zeeman effect due to a misalignment of an anisotropy axis and a magnetic field direction. The ZFS energy is increased in oxidized and reduced states of the molecule indicating enhancement of the anisotropy in these states.

  5. Zero-Magnetic-Field Spin Splitting of Polaron's Ground State Energy Induced by Rashba Spin-Orbit Interaction

    NASA Astrophysics Data System (ADS)

    Liu, Jia; Xiao, Jing-Ling

    2006-10-01

    We study theoretically the ground state energy of a polaron near the interface of a polar-polar semiconductor by considering the Rashba spin-orbit (SO) coupling with the Lee-Low-Pines intermediate coupling method. Our numerical results show that the Rashba SO interaction originating from the inversion asymmetry in the heterostructure splits the ground state energy of the polaron. The electron areal density and vector dependence of the ratio of the SO interaction to the total ground state energy or other energy composition are obvious. One can see that even without any external magnetic field, the ground state energy can be split by the Rashba SO interaction, and this split is not a single but a complex one. Since the presents of the phonons, whose energy gives negative contribution to the polaron's, the spin-splitting states of the polaron are more stable than electron's.

  6. A Perturbation Expansion Method to Study Highly Correlated Spins

    SciTech Connect

    Anda, E. V.; Chiappe, G.; Busser, Carlos A; Davidovich, M. A.; Martins, G. B.; Heidrich-Meisner, F.; Dagotto, Elbio R

    2009-01-01

    This paper proposes a new numerical algorithm to study dynamical spin dependent properties of local highly correlated structures. The method consists in diagonalizing a finite cluster containing the many-body terms of the Hamil- tonian and embedding it into the rest of the system, the Em- bedding Cluster Approximation (ECA), combined with Wil- son s ideas of logarithmic discretization of the representa- tion of the Hamiltonian, the Logarithm Discretization Em- bedded Cluster Approximation (LDECA). The physics as- sociated to a dot and a side-coupled double dot connected to leads are discussed in detail.

  7. Interpretation of the high spin states in Lu161: A paired and unpaired study

    NASA Astrophysics Data System (ADS)

    Ma, Hai-Liang; Carlsson, B. Gillis; Ragnarsson, Ingemar; Ryde, Hans

    2014-07-01

    A paired cranked Nilsson-Strutinsky-Bogoliubov (CNSB) model is presented, which employs the same method to calculate the liquid-drop energy and moment of inertia as the unpaired cranked Nilsson-Strutinsky (CNS) model. In the CNSB model, the energy minimization is carried out in the mesh of pairing gaps Δ and Fermi levels λ as well as deformation parameters. The high spin states in Lu161 are then investigated with the CNSB and CNS models. The terminating structure shows a striking similarity with these two models. Combining the CNSB and CNS models, a complete understanding of high spin structures, including the normal deformed (ND) and triaxial strongly deformed (TSD) bands and observed side bands in Lu161, is achieved. It appears that the only important paired crossings are the first i13/2 neutron crossing and the first h11/2 proton crossing. For the description of the unpaired high spin crossings, it is important to be able to distinguish between the pseudospin partners in the proton N =4 shell, (d5/2,g7/2) and (d3/2,s1/2). The yrast bands are predicted to terminate, which explains the structure of a TSD-like band X2. A band crossing at I ≈36.5 for the TSD band in Lu161, unique within the chain of even-N Lu isotopes, is well described by the CNSB model.

  8. Effects of Exchange Energy and Spin-Orbit Coupling on Bond Energies

    ERIC Educational Resources Information Center

    Smith, Derek W.

    2004-01-01

    Since chemical reactions involve the breaking and making of bonds, understanding the relative strengths of bonds is of paramount importance in the study, teaching, and practice of chemistry. Further, it is showed that free atoms having p(super n) configuration with n = 2,3, or 4 are stabilized by exchange energy, and by spin-orbit coupling for n =…

  9. Inflation in Einstein-Cartan theory with energy-momentum tensor with spin

    NASA Technical Reports Server (NTRS)

    Fennelly, A. J.; Bradas, James C.; Smalley, Larry L.

    1988-01-01

    Generalized, or power-law, inflation is shown to necessarily exist for a simple, anisotropic (Bianchi Type I) cosmology in the Einstein-Cartan gravitational theory with the Ray-Smalley (RS) improved energy-momentum tensor with spin. Formal solution of the EC field equations with the fluid equations of motion explicitly shows inflation caused by the RS spin angular kinetic energy density.

  10. High spin states above the 28{sup {minus}} isomer in {sup 152}Ho

    SciTech Connect

    Rizzutto, M.A.; Ribas, R.V.; Cybulska, E.W.; Oliveira, J.R.; Zahn, G.S.; Medina, N.H.; Bazzacco, D.; Medina, N.H.; Brandolini, F.; Burch, R.; Lunardi, S.; Pavan, P.; Alvarez, C.R.; Spolaore, P.

    1997-03-01

    The structure of the high spin states above the 28{sup {minus}} isomer in the odd-odd {sup 152}Ho nucleus was investigated using the GASP {gamma}-ray spectrometer coupled to the recoil mass spectrometer CAMEL. The {sup 152}Ho nucleus was populated through the {sup 120}Sn({sup 37}Cl,5n) fusion reaction at a beam energy of 187 MeV. A complex level scheme above that isomer was established up to an excitation energy of 13 MeV and I{approx} 40{h_bar}. No rotational bands were observed. {copyright} {ital 1997} {ital The American Physical Society}

  11. Superdeformed band at very high spin in {sup 140}Nd

    SciTech Connect

    Neusser, A.; Huebel, H.; Al-Khatib, A.; Bringel, P.; Buerger, A.; Nenoff, N.; Schoenwasser, G.; Singh, A.K.; Petrache, C.M.; Lo Bianco, G.; Ragnarsson, I.; Hagemann, G.B.; Herskind, B.; Jensen, D.R.; Sletten, G.; Fallon, P.; Goergen, A.; Bednarczyk, P.; Curien, D.; Gangopadhyay, G.

    2004-12-01

    A new high-spin superdeformed band has been discovered in {sub 60}{sup 140}Nd{sub 80}. It was populated in the {sup 96}Zr({sup 48}Ca,4n) reaction and investigated using the EUROBALL {gamma}-ray spectrometer array. The band is observed in the approximate spin range of I=36 to 66. It is associated with shell gaps around Z=60 and at N=80 at large deformation. These gaps produce a pronounced minimum in the calculated total Routhian surfaces at a quadrupole deformation of {epsilon}{sub 2}=0.45. The new band which lies between the high-deformation bands in the A{approx_equal}130 region and the superdeformed bands in A{approx_equal}150 nuclei provides insight into the development of the deformation between these two regions. Two possible configurations are suggested involving four neutrons of i{sub 13/2} origin ({nu}6{sup 4}) and either six protons of h{sub 11/2}/h{sub 9/2} origin ({pi}5{sup 6}) or five protons of h{sub 11/2}/h{sub 9/2} and one of i{sub 13/2} origin ({pi}5{sup 5}6{sup 1})

  12. Control in Highly Focused Top-Spinning. Brief Report.

    ERIC Educational Resources Information Center

    Berkson, Gershon

    1998-01-01

    Three studies analyzed stimulus feedback and the concept of control with three children and two adults having autism. The first study explored feedback from spinning tops, while the second and third emphasized control of various stimuli including spinning tops. Results indicate that autistic individuals' common interest in spinning tops is…

  13. Pressure-driven high to low spin transition in the bimetallic quantum magnet [Ru2(O2CMe)4]3[Cr(CN)6

    SciTech Connect

    O'Neal, K. R.; Liu, Z.; Miller, Joel S.; Fishman, Randy Scott; Musfeldt, J. L.

    2014-01-01

    Synchrotron-based infrared and Raman spectroscopies were brought together with diamond anvil cell techniques and an analysis of the magnetic properties to investigate the pressure-induced high low spin transition in [Ru2(O2CMe)4]3[Cr(CN)6]. The extended nature of the diruthenium wavefunction combined with coupling to chromium-related local lattice distortions changes the relative energies of the and orbitals and drives the high low spin transition on the mixed-valence diruthenium complex. This is a rare example of an externally controlled metamagnetic transition in which both spin-orbit and spin-lattice interactions contribute to the mechanism.

  14. Rashba-Zeeman-effect-induced spin filtering energy windows in a quantum wire

    SciTech Connect

    Xiao, Xianbo Nie, Wenjie; Chen, Zhaoxia; Zhou, Guanghui; Li, Fei

    2014-06-14

    We perform a numerical study on the spin-resolved transport in a quantum wire (QW) under the modulation of both Rashba spin-orbit coupling (SOC) and a perpendicular magnetic field by using the developed Usuki transfer-matrix method in combination with the Landauer-Büttiker formalism. Wide spin filtering energy windows can be achieved in this system for unpolarized spin injection. In addition, both the width of energy window and the magnitude of spin conductance within these energy windows can be tuned by varying Rashba SOC strength, which can be apprehended by analyzing the energy dispersions and spin-polarized density distributions inside the QW, respectively. Further study also demonstrates that these Rashba-SOC-controlled spin filtering energy windows show a strong robustness against disorders. These findings may not only benefit to further understand the spin-dependent transport properties of a QW in the presence of external fields but also provide a theoretical instruction to design a spin filter device.

  15. Energy spectrum and Landau levels in bilayer graphene with spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    Mireles, Francisco; Schliemann, John

    2012-09-01

    We present a theoretical study of the band structure and Landau levels in bilayer graphene at low energies in the presence of a transverse magnetic field and Rashba spin-orbit interaction in the regime of negligible trigonal distortion. Within an effective low-energy approach the (Löwdin partitioning theory), we derive an effective Hamiltonian for bilayer graphene that incorporates the influence of the Zeeman effect, the Rashba spin-orbit interaction and, inclusively, the role of the intrinsic spin-orbit interaction on the same footing. Particular attention is paid to the energy spectrum and Landau levels. Our modeling unveils the strong influence of the Rashba coupling λR in the spin splitting of the electron and hole bands. Graphene bilayers with weak Rashba spin-orbit interaction show a spin splitting linear in momentum and proportional to λR, but scaling inversely proportional to the interlayer hopping energy γ1. However, at robust spin-orbit coupling λR, the energy spectrum shows a strong warping behavior near the Dirac points. We find that the bias-induced gap in bilayer graphene decreases with increasing Rashba coupling, a behavior resembling a topological insulator transition. We further predict an unexpected asymmetric spin splitting and crossings of the Landau levels due to the interplay between the Rashba interaction and the external bias voltage. Our results are of relevance for interpreting magnetotransport and infrared cyclotron resonance measurements, including situations of comparatively weak spin-orbit coupling.

  16. Large-s expansions for the low-energy parameters of the honeycomb-lattice Heisenberg antiferromagnet with spin quantum number s

    NASA Astrophysics Data System (ADS)

    Bishop, R. F.; Li, P. H. Y.

    2016-06-01

    The coupled cluster method (CCM) is employed to very high orders of approximation to study the ground-state (GS) properties of the spin-s Heisenberg antiferromagnet (with isotropic interactions, all of equal strength, between nearest-neighbour pairs only) on the honeycomb lattice. We calculate with high accuracy the complete set of GS parameters that fully describes the low-energy behaviour of the system, in terms of an effective magnon field theory, viz., the energy per spin, the magnetic order parameter (i.e., the sublattice magnetization), the spin stiffness and the zero-field (uniform, transverse) magnetic susceptibility, for all values of the spin quantum numbers in the range 1/2 ≤ s ≤ 9/2. The CCM data points are used to calculate the leading quantum corrections to the classical (s → ∞) values of these low-energy parameters, considered as large-s asymptotic expansions.

  17. Highly selective detection of individual nuclear spins with rotary echo on an electron spin probe

    SciTech Connect

    Mkhitaryan, V. V.; Jelezko, F.; Dobrovitski, V. V.

    2015-10-26

    We consider an electronic spin, such as a nitrogen-vacancy center in diamond, weakly coupled to a large number of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase. We show that by switching the driving phase synchronously with the precession of a given nuclear spin, the interaction to this spin is selectively enhanced, while the rest of the bath remains decoupled. The enhancement is of resonant character. The key feature of the suggested scheme is that the width of the resonance is adjustable, and can be greatly decreased by increasing the driving strength. Thus, the resonance can be significantly narrowed, by a factor of 10–100 in comparison with the existing detection methods. Significant improvement in selectivity is explained analytically and confirmed by direct numerical many-spin simulations. As a result, the method can be applied to a wide range of solid-state systems.

  18. Highly selective detection of individual nuclear spins with rotary echo on an electron spin probe

    DOE PAGESBeta

    Mkhitaryan, V. V.; Jelezko, F.; Dobrovitski, V. V.

    2015-10-26

    We consider an electronic spin, such as a nitrogen-vacancy center in diamond, weakly coupled to a large number of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase. We show that by switching the driving phase synchronously with the precession of a given nuclear spin, the interaction to this spin is selectively enhanced, while the rest of the bath remains decoupled. The enhancement is of resonant character. The key feature of the suggested scheme is that the width of the resonance is adjustable, and can be greatly decreased by increasing the driving strength. Thus, the resonancemore » can be significantly narrowed, by a factor of 10–100 in comparison with the existing detection methods. Significant improvement in selectivity is explained analytically and confirmed by direct numerical many-spin simulations. As a result, the method can be applied to a wide range of solid-state systems.« less

  19. Highly selective detection of individual nuclear spins with rotary echo on an electron spin probe

    PubMed Central

    Mkhitaryan, V. V.; Jelezko, F.; Dobrovitski, V. V.

    2015-01-01

    We consider an electronic spin, such as a nitrogen-vacancy center in diamond, weakly coupled to a large number of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase. We show that by switching the driving phase synchronously with the precession of a given nuclear spin, the interaction to this spin is selectively enhanced, while the rest of the bath remains decoupled. The enhancement is of resonant character. The key feature of the suggested scheme is that the width of the resonance is adjustable, and can be greatly decreased by increasing the driving strength. Thus, the resonance can be significantly narrowed, by a factor of 10–100 in comparison with the existing detection methods. Significant improvement in selectivity is explained analytically and confirmed by direct numerical many-spin simulations. The method can be applied to a wide range of solid-state systems. PMID:26497777

  20. Coexistence of perfect spin filtering for entangled electron pairs and high magnetic storage efficiency in one setup.

    PubMed

    Ji, T T; Bu, N; Chen, F J; Tao, Y C; Wang, J

    2016-01-01

    For Entangled electron pairs superconducting spintronics, there exist two drawbacks in existing proposals of generating entangled electron pairs. One is that the two kinds of different spin entangled electron pairs mix with each other. And the other is a low efficiency of entanglement production. Herein, we report the spin entanglement state of the ferromagnetic insulator (FI)/s-wave superconductor/FI structure on a narrow quantum spin Hall insulator strip. It is shown that not only the high production of entangled electron pairs in wider energy range, but also the perfect spin filtering of entangled electron pairs in the context of no highly spin-polarized electrons, can be obtained. Moreover, the currents for the left and right leads in the antiferromagnetic alignment both can be zero, indicating 100% tunnelling magnetoresistance with highly magnetic storage efficiency. Therefore, the spin filtering for entangled electron pairs and magnetic storage with high efficiencies coexist in one setup. The results may be experimentally demonstrated by measuring the tunnelling conductance and the noise power. PMID:27074893

  1. Coexistence of perfect spin filtering for entangled electron pairs and high magnetic storage efficiency in one setup

    NASA Astrophysics Data System (ADS)

    Ji, T. T.; Bu, N.; Chen, F. J.; Tao, Y. C.; Wang, J.

    2016-04-01

    For Entangled electron pairs superconducting spintronics, there exist two drawbacks in existing proposals of generating entangled electron pairs. One is that the two kinds of different spin entangled electron pairs mix with each other. And the other is a low efficiency of entanglement production. Herein, we report the spin entanglement state of the ferromagnetic insulator (FI)/s-wave superconductor/FI structure on a narrow quantum spin Hall insulator strip. It is shown that not only the high production of entangled electron pairs in wider energy range, but also the perfect spin filtering of entangled electron pairs in the context of no highly spin-polarized electrons, can be obtained. Moreover, the currents for the left and right leads in the antiferromagnetic alignment both can be zero, indicating 100% tunnelling magnetoresistance with highly magnetic storage efficiency. Therefore, the spin filtering for entangled electron pairs and magnetic storage with high efficiencies coexist in one setup. The results may be experimentally demonstrated by measuring the tunnelling conductance and the noise power.

  2. Coexistence of perfect spin filtering for entangled electron pairs and high magnetic storage efficiency in one setup

    PubMed Central

    Ji, T. T.; Bu, N.; Chen, F. J.; Tao, Y. C.; Wang, J.

    2016-01-01

    For Entangled electron pairs superconducting spintronics, there exist two drawbacks in existing proposals of generating entangled electron pairs. One is that the two kinds of different spin entangled electron pairs mix with each other. And the other is a low efficiency of entanglement production. Herein, we report the spin entanglement state of the ferromagnetic insulator (FI)/s-wave superconductor/FI structure on a narrow quantum spin Hall insulator strip. It is shown that not only the high production of entangled electron pairs in wider energy range, but also the perfect spin filtering of entangled electron pairs in the context of no highly spin-polarized electrons, can be obtained. Moreover, the currents for the left and right leads in the antiferromagnetic alignment both can be zero, indicating 100% tunnelling magnetoresistance with highly magnetic storage efficiency. Therefore, the spin filtering for entangled electron pairs and magnetic storage with high efficiencies coexist in one setup. The results may be experimentally demonstrated by measuring the tunnelling conductance and the noise power. PMID:27074893

  3. Unique electron polarimeter analyzing power comparison and precision spin-based energy measurement

    SciTech Connect

    Joseph Grames; Charles Sinclair; Joseph Mitchell; Eugene Chudakov; Howard Fenker; Arne Freyberger; Douglas Higinbotham; B. Poelker; Michael Steigerwald; Michael Tiefenback; Christian Cavata; Stephanie Escoffier; Frederic Marie; Thierry Pussieux; Pascal Vernin; Samuel Danagoulian; Kahanawita Dharmawardane; Renee Fatemi; Kyungseon Joo; Markus Zeier; Viktor Gorbenko; Rakhsha Nasseripour; Brian Raue; Riad Suleiman; Benedikt Zihlmann

    2004-03-01

    Precision measurements of the relative analyzing powers of five electron beam polarimeters, based on Compton, Moller, and Mott scattering, have been performed using the CEBAF accelerator at the Thomas Jefferson National Accelerator Facility (Jefferson Laboratory). A Wien filter in the 100 keV beamline of the injector was used to vary the electron spin orientation exiting the injector. High statistical precision measurements of the scattering asymmetry as a function of the spin orientation were made with each polarimeter. Since each polarimeter receives beam with the same magnitude of polarization, these asymmetry measurements permit a high statistical precision comparison of the relative analyzing powers of the five polarimeters. This is the first time a precise comparison of the analyzing powers of Compton, Moller, and Mott scattering polarimeters has been made. Statistically significant disagreements among the values of the beam polarization calculated from the asymmetry measurements made with each polarimeter reveal either errors in the values of the analyzing power, or failure to correctly include all systematic effects. The measurements reported here represent a first step toward understanding the systematic effects of these electron polarimeters. Such studies are necessary to realize high absolute accuracy (ca. 1%) electron polarization measurements, as required for some parity violation measurements planned at Jefferson Laboratory. Finally, a comparison of the value of the spin orientation exiting the injector that provides maximum longitudinal polarization in each experimental hall leads to an independent and very precise (better than 10-4) absolute measurement of the final electron beam energy.

  4. High-spin spectroscopy in {sup 125}Xe

    SciTech Connect

    Al-Khatib, A.; Bringel, P.; Engelhardt, C.; Huebel, H.; Neusser-Neffgen, A.; Hagemann, G. B.; Sletten, G.; Herskind, B.; Hansen, C. Roenn; Singh, A. K.; Amro, H.; Benzoni, G.; Bracco, A.; Camera, F.; Carpenter, M. P.; Janssens, R. V. F.; Khoo, T. L.; Lauritsen, T.; Chowdhury, P.; Clark, R. M.

    2011-02-15

    Levels excited up to 39.8 MeV and 119/2 units of angular momentum have been populated in {sup 125}Xe by the {sup 82}Se({sup 48}Ca,5n){sup 125}Xe reaction. High-fold {gamma}-ray coincidence events were measured using the Gammasphere Ge detector array. Nine regular rotational bands extending from levels identified previously up to almost 60 ({h_bar}/2{pi}) have been identified, and three of these have been connected to low-lying levels having well-established spins and parities. Configurations have been assigned to six of the bands based on alignment properties, band crossings, and comparison with theoretical cranked shell model calculations (CSM). Transition quadrupole moments have been measured for these bands in the spin range 31-55 ({h_bar}/2{pi}) and were found to be in agreement with the CSM calculations. The corresponding quadrupole deformation {epsilon}{sub 2} ranges from 0.28 to 0.34 at a {gamma} deformation of 0 deg. and from 0.29 to 0.36 at a {gamma} value of 5 deg.

  5. Rapid high-resolution spin- and angle-resolved photoemission spectroscopy with pulsed laser source and time-of-flight spectrometer

    SciTech Connect

    Gotlieb, K.; Hussain, Z.; Bostwick, A.; Jozwiak, C.; Lanzara, A.

    2013-09-15

    A high-efficiency spin- and angle-resolved photoemission spectroscopy (spin-ARPES) spectrometer is coupled with a laboratory-based laser for rapid high-resolution measurements. The spectrometer combines time-of-flight (TOF) energy measurements with low-energy exchange scattering spin polarimetry for high detection efficiencies. Samples are irradiated with fourth harmonic photons generated from a cavity-dumped Ti:sapphire laser that provides high photon flux in a narrow bandwidth, with a pulse timing structure ideally matched to the needs of the TOF spectrometer. The overall efficiency of the combined system results in near-E{sub F} spin-resolved ARPES measurements with an unprecedented combination of energy resolution and acquisition speed. This allows high-resolution spin measurements with a large number of data points spanning multiple dimensions of interest (energy, momentum, photon polarization, etc.) and thus enables experiments not otherwise possible. The system is demonstrated with spin-resolved energy and momentum mapping of the L-gap Au(111) surface states, a prototypical Rashba system. The successful integration of the spectrometer with the pulsed laser system demonstrates its potential for simultaneous spin- and time-resolved ARPES with pump-probe based measurements.

  6. Rhenium-phthalocyanine molecular nanojunction with high magnetic anisotropy and high spin filtering efficiency

    SciTech Connect

    Li, J.; Hu, J.; Wang, H.; Wu, R. Q.

    2015-07-20

    Using the density functional and non-equilibrium Green's function approaches, we studied the magnetic anisotropy and spin-filtering properties of various transition metal-Phthalocyanine molecular junctions across two Au electrodes. Our important finding is that the Au-RePc-Au junction has both large spin filtering efficiency (>80%) and large magnetic anisotropy energy, which makes it suitable for device applications. To provide insights for the further experimental work, we discussed the correlation between the transport property, magnetic anisotropy, and wave function features of the RePc molecule, and we also illustrated the possibility of controlling its magnetic state.

  7. Low temperature and high field regimes of connected kagome artificial spin ice: the role of domain wall topology

    PubMed Central

    Zeissler, Katharina; Chadha, Megha; Lovell, Edmund; Cohen, Lesley F.; Branford, Will R.

    2016-01-01

    Artificial spin ices are frustrated magnetic nanostructures where single domain nanobars act as macrosized spins. In connected kagome artificial spin ice arrays, reversal occurs along one-dimensional chains by propagation of ferromagnetic domain walls through Y-shaped vertices. Both the vertices and the walls are complex chiral objects with well-defined topological edge-charges. At room temperature, it is established that the topological edge-charges determine the exact switching reversal path taken. However, magnetic reversal at low temperatures has received much less attention and how these chiral objects interact at reduced temperature is unknown. In this study we use magnetic force microscopy to image the magnetic reversal process at low temperatures revealing the formation of quite remarkable high energy remanence states and a change in the dynamics of the reversal process. The implication is the breakdown of the artificial spin ice regime in these connected structures at low temperatures. PMID:27443523

  8. HDice, Highly-Polarized Low-Background Frozen-Spin HD Targets for CLAS experiments at Jefferson Lab

    SciTech Connect

    Wei, Xiangdong; Bass, Christopher; D'Angelo, Annalisa; Deur, Alexandre P.; Dezern, Gary L.; Ho, Dao Hoang; Kageya, Tsuneo; Khandaker, Mahbubul A,; Kashy, David H.; Laine, Vivien Eric; Lowry, Michael M.; O'Connell, Thomas Robert; Sandorfi, Andrew M.; Teachey, II, Robert W.; Whisnant, Charles Steven; Zarecky, Michael R.

    2012-12-01

    Large, portable frozen-spin HD (Deuterium-Hydride) targets have been developed for studying nucleon spin properties with low backgrounds. Protons and Deuterons in HD are polarized at low temperatures (~10mK) inside a vertical dilution refrigerator (Oxford Kelvinox-1000) containing a high magnetic field (up to 17T). The targets reach a frozen-spin state within a few months, after which they can be cold transferred to an In-Beam Cryostat (IBC). The IBC, a thin-walled dilution refrigerator operating either horizontally or vertically, is use with quasi-4{pi} detector systems in open geometries with minimal energy loss for exiting reaction products in nucleon structure experiments. The first application of this advanced target system has been used for Spin Sum Rule experiments at the LEGS facility in Brookhaven National Laboratory. An improved target production and handling system has been developed at Jefferson Lab for experiments with the CEBAF Large Acceptance Spectrometer, CLAS.

  9. Low temperature and high field regimes of connected kagome artificial spin ice: the role of domain wall topology.

    PubMed

    Zeissler, Katharina; Chadha, Megha; Lovell, Edmund; Cohen, Lesley F; Branford, Will R

    2016-01-01

    Artificial spin ices are frustrated magnetic nanostructures where single domain nanobars act as macrosized spins. In connected kagome artificial spin ice arrays, reversal occurs along one-dimensional chains by propagation of ferromagnetic domain walls through Y-shaped vertices. Both the vertices and the walls are complex chiral objects with well-defined topological edge-charges. At room temperature, it is established that the topological edge-charges determine the exact switching reversal path taken. However, magnetic reversal at low temperatures has received much less attention and how these chiral objects interact at reduced temperature is unknown. In this study we use magnetic force microscopy to image the magnetic reversal process at low temperatures revealing the formation of quite remarkable high energy remanence states and a change in the dynamics of the reversal process. The implication is the breakdown of the artificial spin ice regime in these connected structures at low temperatures. PMID:27443523

  10. Potential energy curves using unrestricted Møller-Plesset perturbation theory with spin annihilation

    NASA Astrophysics Data System (ADS)

    Schlegel, H. Bernhard

    1986-04-01

    Unrestricted Hartree-Fock and unrestricted Møller-Plesset perturbation theory are convenient methods to compute potential energy curves for bond dissociation, since these methods approach the correct dissociation limit. Unfortunately, a spin unrestricted wave function can contain large contributions from unwanted spin states that can distort the potential energy surface significantly. The spin contamination can be removed by projection or annihilation operators. As is well known, the spin project unrestricted Hartree-Fock bond dissociation curves have a large kink at the onset of the UHF/RHF instability, and a spurious minimum just beyond. However, the spurious minimum disappears and the kink is very much less pronounced at the unrestricted Møller-Plesset level with spin projection. Bond dissociation potentials for LiH and CH4 were computed at the fourth order Møller-Plesset level plus spin projection,4 and good agreement was found with full CI and MR-CISD calculations.

  11. Mass-number and excitation-energy dependence of the spin cutoff parameter

    NASA Astrophysics Data System (ADS)

    Grimes, S. M.; Voinov, A. V.; Massey, T. N.

    2016-07-01

    The spin cutoff parameter determining the nuclear level density spin distribution ρ (J ) is defined through the spin projection as 1 /2 or equivalently for spherical nuclei, ( 3 ) 1 /2. It is needed to divide the total level density into levels as a function of J . To obtain the total level density at the neutron binding energy from the s -wave resonance count, the spin cutoff parameter is also needed. The spin cutoff parameter has been calculated as a function of excitation energy and mass with a super-conducting Hamiltonian. Calculations have been compared with two commonly used semiempirical formulas. A need for further measurements is also observed. Some complications for deformed nuclei are discussed. The quality of spin cut off parameter data derived from isomeric ratio measurement is examined.

  12. High-pressure magic angle spinning nuclear magnetic resonance

    SciTech Connect

    Hoyt, David W.; Turcu, Romulus V. F.; Sears, Jesse A.; Rosso, Kevin M.; Burton, Sarah D.; Felmy, Andrew R.; Hu, Jian Zhi

    2011-10-01

    A high-pressure magic angle spinning (MAS) NMR capability, consisting of a reusable high-pressure MAS rotor, a high-pressure rotor loading/reaction chamber for in situ sealing and re-opening of the high-pressure MAS rotor, and a MAS probe with a localized RF coil for background signal suppression, is reported. The unusual technical challenges associated with development of a reusable high-pressure MAS rotor are addressed in part by modifying standard ceramics for the rotor sleeve by abrading the internal surface at both ends of the cylinder. In this way, not only is the advantage of ceramic cylinders for withstanding very high-pressure utilized, but also plastic bushings can be glued tightly in place so that other removable plastic sealing mechanisms/components and O-rings can be mounted to create the desired high-pressure seal. Using this strategy, sealed internal pressures exceeding 150 bars have been achieved and sustained under ambient external pressure with minimal loss of pressure for 72 h. Finally, as an application example, in situ13C MAS NMR studies of mineral carbonation reaction intermediates and final products of forsterite (Mg2SiO4) reacted with supercritical CO2 and H2O at 150 bar and 50 °C are reported, with relevance to geological sequestration of carbon dioxide.

  13. High-pressure magic angle spinning nuclear magnetic resonance.

    PubMed

    Hoyt, David W; Turcu, Romulus V F; Sears, Jesse A; Rosso, Kevin M; Burton, Sarah D; Felmy, Andrew R; Hu, Jian Zhi

    2011-10-01

    A high-pressure magic angle spinning (MAS) NMR capability, consisting of a reusable high-pressure MAS rotor, a high-pressure rotor loading/reaction chamber for in situ sealing and re-opening of the high-pressure MAS rotor, and a MAS probe with a localized RF coil for background signal suppression, is reported. The unusual technical challenges associated with development of a reusable high-pressure MAS rotor are addressed in part by modifying standard ceramics for the rotor sleeve by abrading the internal surface at both ends of the cylinder. In this way, not only is the advantage of ceramic cylinders for withstanding very high-pressure utilized, but also plastic bushings can be glued tightly in place so that other removable plastic sealing mechanisms/components and O-rings can be mounted to create the desired high-pressure seal. Using this strategy, sealed internal pressures exceeding 150 bars have been achieved and sustained under ambient external pressure with minimal loss of pressure for 72 h. As an application example, in situ(13)C MAS NMR studies of mineral carbonation reaction intermediates and final products of forsterite (Mg(2)SiO(4)) reacted with supercritical CO(2) and H(2)O at 150 bar and 50°C are reported, with relevance to geological sequestration of carbon dioxide. PMID:21862372

  14. High-pressure magic angle spinning nuclear magnetic resonance

    NASA Astrophysics Data System (ADS)

    Hoyt, David W.; Turcu, Romulus V. F.; Sears, Jesse A.; Rosso, Kevin M.; Burton, Sarah D.; Felmy, Andrew R.; Hu, Jian Zhi

    2011-10-01

    A high-pressure magic angle spinning (MAS) NMR capability, consisting of a reusable high-pressure MAS rotor, a high-pressure rotor loading/reaction chamber for in situ sealing and re-opening of the high-pressure MAS rotor, and a MAS probe with a localized RF coil for background signal suppression, is reported. The unusual technical challenges associated with development of a reusable high-pressure MAS rotor are addressed in part by modifying standard ceramics for the rotor sleeve by abrading the internal surface at both ends of the cylinder. In this way, not only is the advantage of ceramic cylinders for withstanding very high-pressure utilized, but also plastic bushings can be glued tightly in place so that other removable plastic sealing mechanisms/components and O-rings can be mounted to create the desired high-pressure seal. Using this strategy, sealed internal pressures exceeding 150 bars have been achieved and sustained under ambient external pressure with minimal loss of pressure for 72 h. As an application example, in situ13C MAS NMR studies of mineral carbonation reaction intermediates and final products of forsterite (Mg 2SiO 4) reacted with supercritical CO 2 and H 2O at 150 bar and 50 °C are reported, with relevance to geological sequestration of carbon dioxide.

  15. Equation-of-motion coupled cluster method for the description of the high spin excited states.

    PubMed

    Musiał, Monika; Lupa, Łukasz; Kucharski, Stanisław A

    2016-04-21

    The equation-of-motion (EOM) coupled cluster (CC) approach in the version applicable for the excitation energy(EE) calculations has been formulated for high spin components. The EE-EOM-CC scheme based on the restricted Hartree-Fock reference and standard amplitude equations as used in the Davidson diagonalization procedure yields the singlet states. The triplet and higher spin components require separate amplitude equations. In the case of quintets, the relevant equations are much simpler and easier to solve. Out of 26 diagrammatic terms contributing to the R1 and R2 singlet equations in the case of quintets, only R2 operator survives with 5 diagrammatic terms present. In addition all terms engaging three body elements of the similarity transformed Hamiltonian disappear. This indicates a substantial simplification of the theory. The implemented method has been applied to the pilot study of the excited states of the C2 molecule and quintet states of C and Si atoms. PMID:27389207

  16. Equation-of-motion coupled cluster method for the description of the high spin excited states

    NASA Astrophysics Data System (ADS)

    Musiał, Monika; Lupa, Łukasz; Kucharski, Stanisław A.

    2016-04-01

    The equation-of-motion (EOM) coupled cluster (CC) approach in the version applicable for the excitation energy (EE) calculations has been formulated for high spin components. The EE-EOM-CC scheme based on the restricted Hartree-Fock reference and standard amplitude equations as used in the Davidson diagonalization procedure yields the singlet states. The triplet and higher spin components require separate amplitude equations. In the case of quintets, the relevant equations are much simpler and easier to solve. Out of 26 diagrammatic terms contributing to the R1 and R2 singlet equations in the case of quintets, only R2 operator survives with 5 diagrammatic terms present. In addition all terms engaging three body elements of the similarity transformed Hamiltonian disappear. This indicates a substantial simplification of the theory. The implemented method has been applied to the pilot study of the excited states of the C2 molecule and quintet states of C and Si atoms.

  17. Low-energy-state dynamics of entanglement for spin systems

    SciTech Connect

    Jafari, R.

    2010-11-15

    We develop the ideas of the quantum renormalization group and quantum information by exploring the low-energy-state dynamics of entanglement resources of a system close to its quantum critical point. We demonstrate that low-energy-state dynamical quantities of one-dimensional magnetic systems can show a quantum phase transition point and show scaling behavior in the vicinity of the transition point. To present our idea, we study the evolution of two spin entanglements in the one-dimensional Ising model in the transverse field. The system is initialized as the so-called thermal ground state of the pure Ising model. We investigate the evolution of the generation of entanglement with increasing magnetic field. We obtain that the derivative of the time at which the entanglement reaches its maximum with respect to the transverse field diverges at the critical point and its scaling behaviors versus the size of the system are the same as the static ground-state entanglement of the system.

  18. High-efficiency spin-resolved and spin-integrated electron detection: Parallel mounting on a hemispherical analyzer

    NASA Astrophysics Data System (ADS)

    Ghiringhelli, G.; Larsson, K.; Brookes, N. B.

    1999-11-01

    We have mounted a compact 25 kV mini-Mott spin polarimeter on a commercial high-throughput hemispherical electron analyzer with a double purpose: to maximize the polarization detection and to preserve the original efficiency of the spectrometer in the spin-integrated measurements. We have thus replaced the 16-anode microchannel-plate detector with a 12-anode microsphere-plate detector in parallel with a Rice University retarding Mott spin polarimeter. Passing from one detection mode to the other is quick and easy. The transfer optics from the analyzer exit slit to the scattering target of the polarimeter allows the full potential of both the electron analyzer and the spin detector to be exploited. The expected effective Sherman function (Seff=0.17) and figure of merit (η0≅1.4×10-4) are found in the spin-resolved mode, and only 25% of the original efficiency is lost in the spin-integrated acquisitions.

  19. Spin-symmetry conversion and internal rotation in high J molecular systems

    NASA Astrophysics Data System (ADS)

    Mitchell, Justin; Harter, William

    2006-05-01

    Dynamics and spectra of molecules with internal rotation or rovibrational coupling is approximately modeled by rigid or semi-rigid rotors with attached gyroscopes. Using Rotational Energy (RE)^1 surfaces, high resolution molecular spectra for high angular momentum show two distinct but related phenomena; spin-symmetry conversion and internal rotation. For both cases the high total angular momentum allows for transitions that would otherwise be forbidden. Molecular body-frame J-localization effects associated with tight energy level-clusters dominate the rovibronic spectra of high symmetry molecules, particularly spherical tops at J>10. ^2 The effects include large and widespread spin-symmetry mixing contrary to conventional wisdom^3 about weak nuclear moments. Such effects are discussed showing how RE surface plots may predict them even at low J. Classical dynamics of axially constrained rotors are approximated by intersecting rotational-energy-surfaces (RES) that have (J-S).B.(J-S) forms in the limit of constraints that do no work. Semi-classical eigensolutions are compared to those found by direct diagonalization. ^1 W.G Hater, in Handbook of Atomic, Molecular and Optical Physics, edited by G.W.F Drake (Springer, Germany 2006) ^2 W. G. Harter, Phys. Rev. A24,192-262(1981). ^3 G. Herzberg, Infrared and Raman Spectra (VanNostrand 1945) pp. 458,463.

  20. A 3D-Printed High Power Nuclear Spin Polarizer

    PubMed Central

    Nikolaou, Panayiotis; Coffey, Aaron M.; Walkup, Laura L.; Gust, Brogan M.; LaPierre, Cristen D.; Koehnemann, Edward; Barlow, Michael J.; Rosen, Matthew S.; Goodson, Boyd M.; Chekmenev, Eduard Y.

    2015-01-01

    Three-dimensional printing with high-temperature plastic is used to enable spin exchange optical pumping (SEOP) and hyperpolarization of xenon-129 gas. The use of 3D printed structures increases the simplicity of integration of the following key components with a variable temperature SEOP probe: (i) in situ NMR circuit operating at 84 kHz (Larmor frequencies of 129Xe and 1H nuclear spins), (ii) <0.3 nm narrowed 200 W laser source, (iii) in situ high-resolution near-IR spectroscopy, (iv) thermoelectric temperature control, (v) retroreflection optics, and (vi) optomechanical alignment system. The rapid prototyping endowed by 3D printing dramatically reduces production time and expenses while allowing reproducibility and integration of “off-the-shelf” components and enables the concept of printing on demand. The utility of this SEOP setup is demonstrated here to obtain near-unity 129Xe polarization values in a 0.5 L optical pumping cell, including ~74 ± 7% at 1000 Torr xenon partial pressure, a record value at such high Xe density. Values for the 129Xe polarization exponential build-up rate [(3.63 ± 0.15) × 10−2 min−1] and in-cell 129Xe spin−lattice relaxation time (T1 = 2.19 ± 0.06 h) for 1000 Torr Xe were in excellent agreement with the ratio of the gas-phase polarizations for 129Xe and Rb (PRb ~ 96%). Hyperpolarization-enhanced 129Xe gas imaging was demonstrated with a spherical phantom following automated gas transfer from the polarizer. Taken together, these results support the development of a wide range of chemical, biochemical, material science, and biomedical applications. PMID:24400919

  1. The spin-polaron theory of high-Tc superconductivity

    NASA Astrophysics Data System (ADS)

    Mott, N. F.

    1990-01-01

    An outline is given of the model for some high-temperature superconductors which assumes that the carriers are holes in the (hybridized) oxygen 2p band and form ‘spin polarons’ with the moments on the copper atoms. A comparison is made with observations of spin polarons in Gd3-xvxS4 and with the properties of La1-xSrxVO3 in relation to those of La2-xSrxCuO4. It is assumed, following several authors, that in the superconductors the polarons form bipolarons, which are bosons, and a comparison is made with some other treatments of this hypothesis. It is proposed that in many such superconductors the boson, essentially a pair of these holes, moves in an impurity band, and that normally all the polarons (fermions) form bipolarons; the fermions repel each other on the same site (positive Hubbard U) but attract when on adjacent sites; the critical temperature Tc is then that at which the Bose gas becomes non-degenerate. In such materials a non-degenerate gas of bosons would carry the current above Tc as first suggested by Alexandrov et al. (1986). The linear increase in the resistivity above Tc is explained on this hypothesis. The effective mass of the bipolaron is, we believe, large (˜20 30me). The copper 3d9 moments in the superconducting range resonate between their two orientations as a consequence of the motion of the carriers, as they do in the description by Brinkman and Rice (1970) of highly correlated metals. Spin polarons, we believe, form only when this is so, but not in the antiferromagnetic range of x. A discussion is given of the resistivity above Tc, thermopower above Tc, and of the nature of the superconducting gap as shown by tunnelling. We confine our discussion to the materials containing copper, excluding for instance cubic Ba1-xKxBiO3, and possibly any superconductor containing bismuth, where the bosons may be Bi3+.

  2. Spin-resolved photoelectron spectroscopy using femtosecond extreme ultraviolet light pulses from high-order harmonic generation.

    PubMed

    Plötzing, M; Adam, R; Weier, C; Plucinski, L; Eich, S; Emmerich, S; Rollinger, M; Aeschlimann, M; Mathias, S; Schneider, C M

    2016-04-01

    The fundamental mechanism responsible for optically induced magnetization dynamics in ferromagnetic thin films has been under intense debate since almost two decades. Currently, numerous competing theoretical models are in strong need for a decisive experimental confirmation such as monitoring the triggered changes in the spin-dependent band structure on ultrashort time scales. Our approach explores the possibility of observing femtosecond band structure dynamics by giving access to extended parts of the Brillouin zone in a simultaneously time-, energy- and spin-resolved photoemission experiment. For this purpose, our setup uses a state-of-the-art, highly efficient spin detector and ultrashort, extreme ultraviolet light pulses created by laser-based high-order harmonic generation. In this paper, we present the setup and first spin-resolved spectra obtained with our experiment within an acquisition time short enough to allow pump-probe studies. Further, we characterize the influence of the excitation with femtosecond extreme ultraviolet pulses by comparing the results with data acquired using a continuous wave light source with similar photon energy. In addition, changes in the spectra induced by vacuum space-charge effects due to both the extreme ultraviolet probe- and near-infrared pump-pulses are studied by analyzing the resulting spectral distortions. The combination of energy resolution and electron count rate achieved in our setup confirms its suitability for spin-resolved studies of the band structure on ultrashort time scales. PMID:27131684

  3. Spin-resolved photoelectron spectroscopy using femtosecond extreme ultraviolet light pulses from high-order harmonic generation

    NASA Astrophysics Data System (ADS)

    Plötzing, M.; Adam, R.; Weier, C.; Plucinski, L.; Eich, S.; Emmerich, S.; Rollinger, M.; Aeschlimann, M.; Mathias, S.; Schneider, C. M.

    2016-04-01

    The fundamental mechanism responsible for optically induced magnetization dynamics in ferromagnetic thin films has been under intense debate since almost two decades. Currently, numerous competing theoretical models are in strong need for a decisive experimental confirmation such as monitoring the triggered changes in the spin-dependent band structure on ultrashort time scales. Our approach explores the possibility of observing femtosecond band structure dynamics by giving access to extended parts of the Brillouin zone in a simultaneously time-, energy- and spin-resolved photoemission experiment. For this purpose, our setup uses a state-of-the-art, highly efficient spin detector and ultrashort, extreme ultraviolet light pulses created by laser-based high-order harmonic generation. In this paper, we present the setup and first spin-resolved spectra obtained with our experiment within an acquisition time short enough to allow pump-probe studies. Further, we characterize the influence of the excitation with femtosecond extreme ultraviolet pulses by comparing the results with data acquired using a continuous wave light source with similar photon energy. In addition, changes in the spectra induced by vacuum space-charge effects due to both the extreme ultraviolet probe- and near-infrared pump-pulses are studied by analyzing the resulting spectral distortions. The combination of energy resolution and electron count rate achieved in our setup confirms its suitability for spin-resolved studies of the band structure on ultrashort time scales.

  4. Highly reliable spin-coated titanium dioxide dielectric

    NASA Astrophysics Data System (ADS)

    Mondal, Sandip; Kumar, Arvind; Rao, K. S. R. Koteswara; Venkataraman, V.

    2016-05-01

    Dielectric degradation as low as 0.3 % has been observed for a highly reliable Titanium dioxide (TiO2) film after constant voltage stressing (CVS) with - 4 V for 105 second at room temperature (300 K). The film was fabricated by sol -gel spin - coating method on a lightly doped p-Si (~1015 cm-3) substrate. The equivalent oxide thickness (EOT) is 7 nm with a dielectric constant 33 (at 1 MHz). Metal - Oxide - Semiconductor (MOS) capacitors have been fabricated with an optimum annealing temperature of 800°C for one hour in a preheated furnace. The dielectric degradation is annealing temperature dependent. A degradation of 1.4 %, 1.2 % and 1.1 % has been observed for 400°C, 600°C and 1000°C temperature annealed MOS respectively. The dielectric degradation increases below or above the optimum temperature of annealing.

  5. High power Nd:YAG spinning disk laser.

    PubMed

    Ongstad, Andrew P; Guy, Matthew; Chavez, Joeseph R

    2016-01-11

    We report on a high power Nd:YAG spinning disk laser. The eight cm diameter disk generated 200 W CW output with 323 W of absorbed pump in a near diffraction-limited beam. The power conversion efficiency was 64%. The pulsed result, 5 ms pulses at 10 Hz PRF, was nearly identical to the CW result indicating good thermal management. Rotated at 1200-1800 RPM with He impingement cooling the disk temperature increased by only 17 °C reaching a maximum temperature of ~31 °C. The thermal dissipation per unit of output power was 0.61 watt of heat generated per watt of laser output, which is below the typical range of 0.8-1.1 for 808 nm diode pumped Nd:YAG lasers. PMID:26832242

  6. High-energy detector

    DOEpatents

    Bolotnikov, Aleksey E.; Camarda, Giuseppe; Cui, Yonggang; James, Ralph B.

    2011-11-22

    The preferred embodiments are directed to a high-energy detector that is electrically shielded using an anode, a cathode, and a conducting shield to substantially reduce or eliminate electrically unshielded area. The anode and the cathode are disposed at opposite ends of the detector and the conducting shield substantially surrounds at least a portion of the longitudinal surface of the detector. The conducting shield extends longitudinally to the anode end of the detector and substantially surrounds at least a portion of the detector. Signals read from one or more of the anode, cathode, and conducting shield can be used to determine the number of electrons that are liberated as a result of high-energy particles impinge on the detector. A correction technique can be implemented to correct for liberated electron that become trapped to improve the energy resolution of the high-energy detectors disclosed herein.

  7. Adsorption energy and spin state of first-row transition metals adsorbed on MgO(100)

    NASA Astrophysics Data System (ADS)

    Markovits, A.; Paniagua, J. C.; López, N.; Minot, C.; Illas, F.

    2003-03-01

    Slab and cluster model spin-polarized calculations have been carried out to study various properties of isolated first-row transition metal atoms adsorbed on the anionic sites of the regular MgO(100) surface. The calculated adsorption energies follow the trend of the metal cohesive energies, indicating that the changes in the metal-support and metal-metal interactions along the series are dominated by atomic properties. In all cases, except for Ni at the generalized gradient approximation level, the number of unpaired electron is maintained as in the isolated metal atom. The energy required to change the atomic state from high to low spin has been computed using the PW91 and B3LYP density-functional-theory-based methods. PW91 fails to predict the proper ground state of V and Ni, but the results for the isolated and adsorbed atom are consistent within the method. B3LYP properly predicts the ground state of all first-row transition atom the high- to low-spin transition considered is comparable to experiment. In all cases, the interaction with the surface results in a reduced high- to low-spin transition energy.

  8. Decoupling a spin qubit from high-frequency Larmor dynamics of a GaAs nuclear spin bath

    NASA Astrophysics Data System (ADS)

    Malinowski, Filip K.; Martins, Frederico; Nissen, Peter D.; Rudner, Mark S.; Marcus, Charles M.; Kuemmeth, Ferdinand; Barnes, Edwin; Fallahi, Saeed; Gardner, Geoffrey C.; Manfra, Michael J.

    We present a technique of decoupling a spin qubit in a GaAs/AlGaAs heterostructure from low- and high-frequency noise arising from hyperfine interaction of electrons with nuclear spins. We use Carr-Purcell-Meiboom-Gill sequences in which we synchronize the repetition rate of π pulses to difference Larmor frequencies of 69Ga, 71Ga and 75As nuclei. This decouples the qubit both from low-frequency noise due to diffusion of nuclear spins and from noise at selected high frequencies, allowing us to apply more than a thousand π pulses in a sequence. We demonstrate a coherence time of a singlet-triplet qubit of 0.87 ms, i.e. five orders of magnitude longer than the inhomogeneous dephasing time intrinsic to GaAs. Support through IARPA-MQCO, Army Research Office, LPS-MPO-CMTC, the Villum Foundation and the Danish National Research Foundation is acknowledged.

  9. Spin stability of sounding rocket secondary payloads following high velocity ejections

    NASA Astrophysics Data System (ADS)

    Nelson, Weston M.

    The Auroral Spatial Structures Probe (ASSP) mission is a sounding rocket mission studying solar energy input to space weather. ASSP requires the high velocity ejection (up to 50 m/s) of 6 secondary payloads, spin stabilized perpendicular to the ejection velocity. The proposed scientific instrumentation depends on a high degree of spin stability, requiring a maximum coning angle of less than 5°. It also requires that the spin axis be aligned within 25° of the local magnetic field lines. The maximum velocities of current ejection methods are typically less than 10m/s, and often produce coning angles in excess of 20°. Because of this they do not meet the ASSP mission requirements. To meet these requirements a new ejection method is being developed by NASA Wallops Flight Facility. Success of the technique in meeting coning angle and B-field alignment requirements is evaluated herein by modeling secondary payload dynamic behavior using a 6-DOF dynamic simulation employing state space integration written in MATLAB. Simulation results showed that secondary payload mass balancing is the most important factor in meeting stability requirements. Secondary mass payload properties will be measured using an inverted torsion pendulum. If moment of inertia measurement errors can be reduced to 0.5%, it is possible to achieve mean coning and B-field alignment angles of 2.16° and 2.71°, respectively.

  10. Controlled tunneling-induced dephasing of Rabi rotations for high-fidelity hole spin initialization

    NASA Astrophysics Data System (ADS)

    Ardelt, P.-L.; Simmet, T.; Müller, K.; Dory, C.; Fischer, K. A.; Bechtold, A.; Kleinkauf, A.; Riedl, H.; Finley, J. J.

    2015-09-01

    We report the subpicosecond initialization of a single heavy hole spin in a self-assembled quantum dot with >98.5 % fidelity and without external magnetic field. Using an optically addressable charge and spin storage device we tailor the relative electron and hole tunneling escape time scales from the dot and simultaneously achieve high-fidelity initialization, long hole storage times, and high-efficiency readout via a photocurrent signal. We measure electric-field-dependent Rabi oscillations of the neutral and charged exciton transitions in the ultrafast tunneling regime and demonstrate that tunneling-induced dephasing (TID) of excitonic Rabi rotations is the major source for the intensity damping of Rabi oscillations in the low Rabi frequency, low temperature regime. Our results are in very good quantitative agreement with quantum-optical simulations revealing that TID can be used to precisely measure tunneling escape times and extract changes in the Coulomb binding energies for different charge configurations of the quantum dot. Finally, we demonstrate that for subpicosecond electron tunneling escape, TID of a coherently driven exciton transition facilitates ultrafast hole spin initialization with near-unity fidelity.

  11. High energy beam lines

    NASA Astrophysics Data System (ADS)

    Marchetto, M.; Laxdal, R. E.

    2014-01-01

    The ISAC post accelerator comprises an RFQ, DTL and SC-linac. The high energy beam lines connect the linear accelerators as well as deliver the accelerated beams to two different experimental areas. The medium energy beam transport (MEBT) line connects the RFQ to the DTL. The high energy beam transport (HEBT) line connects the DTL to the ISAC-I experimental stations (DRAGON, TUDA-I, GPS). The DTL to superconducting beam (DSB) transport line connects the ISAC-I and ISAC-II linacs. The superconducting energy beam transport (SEBT) line connects the SC linac to the ISAC-II experimental station (TUDA-II, HERACLES, TIGRESS, EMMA and GPS). All these lines have the function of transporting and matching the beams to the downstream sections by manipulating the transverse and longitudinal phase space. They also contain diagnostic devices to measure the beam properties.

  12. Two Energy Scales in the Spin Excitations of La2-xSrxCu04

    NASA Astrophysics Data System (ADS)

    Hayden, Stephen

    2007-03-01

    There has recently been considerable progress in electronic quasiparticle spectroscopy of high-Tc superconductors. Angle resolved photoemission and tunnelling indicate that the quasiparticles are strongly coupled to excitations with energies in the range 40-70 meV. The recent debate has focused around phonons being the coupled excitations. The focus on phonons is largely because high-resolution phonon spectra are available and they contain considerable structure. Collective spin excitations are promising candidates for the strongly coupled excitations. However high resolution neutron data in the relevant 40-70 meV energy range have not been available for compounds where the quasiparticle anomalies are observed. In order to fill this gap in our knowledge, we have prepared 50g of single crystals of La1.84Sr0.16CuO4 and carried out a new study of the magnetic excitations over a wide energy range, with considerably better energy resolution than our previous studies, and with good momentum resolution. Experiments were carried out using the MAPS spectrometer at the ISIS spallation neutron source. Our results demonstrate that the magnetic excitations have a two component structure with a low-frequency component strongest around 18 meV and a broader component strongest near 40-70 meV. The second component carries most of the spectral weight and its energy matches structure seen in photoemission and tunnelling spectra in the range 50-90 meV. Thus collective spin excitations may explain features of quasiparticle spectroscopies and are therefore likely to be strongly coupled excitations. The high-frequency excitations are most naturally interpreted as being due to residual antiferromagnetic interactions. [1] e.g. A. Lanzara, Nature 412, p510 (2001) [2] e.g. J Lee et al., Nature 442, p546 (2006)

  13. In-Beam Studies of High Spin States in Mercury -182 and MERCURY-184

    NASA Astrophysics Data System (ADS)

    Bindra, Kanwarjit Singh

    The high spin states in ^{182 }Hg were studied by using the reaction ^{154}Gd(^{32}S, 4n) at the Holifield Heavy Ion Research Facility. In addition, the in-beam gamma-rays in ^{183}Hg were identified for the first time using the reaction ^{155}Gd(^{32}S, 4n) at the Argonne BGO-FMA facility. Five new bands were observed for the first time in ^{182}Hg by studying the gamma-gamma coincidence relationships. The spins and parities of the nuclear levels were assigned on the basis of the measured ratios of directional correlations for oriented nuclei (DCO ratios). Shape co-existence similar to that observed in ^{184{-}186}Hg was established. The well deformed prolate band was extended to a state with tentative spin (20^+). The 2^+ state of the prolate band was identified at an energy of 548.6 keV which is higher in energy than in ^{184}Hg. A two parameter band mixing calculation yielded an interaction strength of 87 keV between the prolate 2^+ and the oblate 2^+ states. Four of the five new bands were found to be similar in behavior to ones seen in ^{184}Hg. An attempt was made to study the behavior of some of these bands at high spins by analyzing their kinematic and dynamic moments of inertia. The gamma-ray transitions in ^{183}Hg were identified from fragment-gamma and gamma-gamma coincidence measurements. A total of five bands of levels were identified and the spins and parities of the levels were assigned by comparing the level scheme of ^{138 }Hg obtained with that of ^ {185}Hg established previously. The interpretation of these bands in terms of associated quasi-particle configurations also relies on noted similarities with the structure of ^{185}Hg. Shape co-existence was established in ^{183}Hg as a result of this study. Two of the bands associated with the (624) 9/2^+ orbital were found to exhibit signature splitting, as expected for i _{13/2} excitations built on the prolate shape with moderate deformation. Two other bands which do not show signature splitting

  14. High precision measurements of the neutron spin structure in Hall A at Jlab

    SciTech Connect

    Annand, R M; Cates, G; Cisbani, E; Franklin, G B; Liyanage, N; Puckett, A; Rosner, G; Wojtsekhowski, B; Zheng, X

    2012-04-01

    Conclusions of this presentation are: (1) JLab energy upgrade will offer new exciting opportunities to study the nucleon (spin) structure such as high precision, unexplored phase space, flavor decomposition; (2) Large technological efforts is in progress to optimally exploit these opportunities; (3) HallA will be the first hall to get the new beam, first experiment expected to run in 2014; (4) A1n likely one of the first experiments to take data in the new 12 GeV era; and (5) SIDIS exp. will follow in couple of years.

  15. Fusion with highly spin polarized HD and D sub 2

    SciTech Connect

    Honig, A.

    1992-06-29

    This report discusses the following topics relating to inertial confinement with spin polarized hydrogen targets: low temperature implementation of mating a target to omega; dilution-refrigerator cold-entry and retrieval system; target shell tensile strength characterization at low temperatures; and proton and deuteron spin-lattice relaxation measurements in HD in the millikelvin temperature range. (LSP)

  16. Complete protocol for slow-spinning high-resolution magic-angle spinning NMR analysis of fragile tissues.

    PubMed

    André, Marion; Dumez, Jean-Nicolas; Rezig, Lamya; Shintu, Laetitia; Piotto, Martial; Caldarelli, Stefano

    2014-11-01

    High-resolution magic-angle spinning (HR-MAS) nuclear magnetic resonance (NMR) is an essential tool to characterize a variety of semisolid systems, including biological tissues, with virtually no sample preparation. The "non-destructive" nature of NMR is typically compromised, however, by the extreme centrifugal forces experienced under conventional HR-MAS frequencies of several kilohertz. These features limit the usefulness of current HR-MAS approaches for fragile samples. Here, we introduce a full protocol for acquiring high-quality HR-MAS NMR spectra of biological tissues at low spinning rates (down to a few hundred hertz). The protocol first consists of a carefully designed sample preparation, which yields spectra without significant spinning sidebands at low spinning frequency for several types of sample holders, including the standard disposable inserts classically used in HR-MAS NMR-based metabolomics. Suppression of broad spectral features is then achieved using a modified version of the recently introduced PROJECT experiment with added water suppression and rotor synchronization, which deposits limited power in the sample and which can be suitably rotor-synchronized at low spinning rates. The performance of the slow HR-MAS NMR procedure is demonstrated on conventional (liver tissue) and very delicate (fish eggs) samples, for which the slow-spinning conditions are shown to preserve the structural integrity and to minimize intercompartmental leaks of metabolites. Taken together, these results expand the applicability and reliability of HR-MAS NMR spectroscopy. These results have been obtained at 400 and 600 MHz and suggest that high-quality slow HR-MAS spectra can be expected at higher magnetic fields using the described protocol. PMID:25286333

  17. High Energy Astrophysics Program

    NASA Technical Reports Server (NTRS)

    1996-01-01

    This report reviews activities performed by members of the USRA (Universities Space Research Association) contract team during the six months during the reporting period (10/95 - 3/96) and projected activities during the coming six months. Activities take place at the Goddard Space Flight Center, within the Laboratory for High Energy Astrophysics. Developments concern instrumentation, observation, data analysis, and theoretical work in Astrophysics. Missions supported include: Advanced Satellite for Cosmology and Astrophysics (ASCA), X-ray Timing Experiment (XTE), X-ray Spectrometer (XRS), Astro-E, High Energy Astrophysics Science, Archive Research Center (HEASARC), and others.

  18. High Energy Astrophysics Program

    NASA Technical Reports Server (NTRS)

    1996-01-01

    This report reviews activities performed-by members of the USRA contract team during the six months of the reporting period and projected activities during the coming six months. Activities take place at the Goddard Space Flight Center, visiting the Laboratory for High Energy Astrophysics. Developments concern instrumentation, observation, data analysis, and theoretical work in Astrophysics. Missions supported include: Advanced Satellite for Cosmology and Astrophysics (ASCA); X-ray Timing Experiment (XTE); X-ray Spectrometer (XRS); Astro-E; High Energy Astrophysics Science Archive Research Center (HEASARC), and others.

  19. Solute-Solvent Interactions and High Spin ⇌ Low Spin Transitions in Ferric Dithiocarbamates

    NASA Astrophysics Data System (ADS)

    Ganguli, P.

    1985-01-01

    The HS ⇌ LS transition in ferric dithiocarbamates in a number of solvents has been investigated using NMR and is interpreted in terms of preferential solvation or second co-ordination sphere reorganisation effects. These studies clearly demonstrate that neglect of pseudo contact shifts can lead to erroneous conclusions about the spin delocalisation mechanisms. The spin derealization in these systems is by direct σ-delocalization along the alkyl chain. The As values of 2T2 and 6A1 states have the same sign.

  20. Spectroscopy and high-spin structure of {sup 209}Fr

    SciTech Connect

    Dracoulis, G. D.; Davidson, P. M.; Lane, G. J.; Kibedi, T.; Nieminen, P.; Watanabe, H.; Byrne, A. P.; Wilson, A. N.

    2009-05-15

    Excited states in {sup 209}Fr have been studied using the {sup 197}Au({sup 16}O,4n){sup 209}Fr reaction with pulsed beams and {gamma}-ray and electron spectroscopy. A comprehensive scheme has been established up to an excitation energy of about 6 MeV and spins of about 49/2({Dirac_h}/2{pi}). Several isomers have been identified including a J{sup {pi}}=25/2{sup +}, {tau}=48(3) ns state at 2130 keV and a 606(26) ns, 45/2{sup -} state at 4660 keV. The latter state decays via an enhanced E3 transition with a strength of 28.8(12) W.u. It can be identified with a similar isomer in the heavier odd isotopes {sup 211}Fr and {sup 213}Fr, arising from the maximal coupling of the five valence protons in the {pi}h{sub 9/2}{sup 3}i{sub 13/2}{sup 2} configuration. The systematics of the yrast states in the odd-A isotopes are discussed, including the presence of states arising from the main proton configurations coupled to the p{sub 1/2}, f{sub 5/2}, and i{sub 13/2} neutron holes. Shell-model configurations are assigned to many of the observed states. The isotopic assignment differs from earlier work, which is shown to be erroneous.

  1. High-fidelity gates in quantum dot spin qubits

    PubMed Central

    Koh, Teck Seng; Coppersmith, S. N.; Friesen, Mark

    2013-01-01

    Several logical qubits and quantum gates have been proposed for semiconductor quantum dots controlled by voltages applied to top gates. The different schemes can be difficult to compare meaningfully. Here we develop a theoretical framework to evaluate disparate qubit-gating schemes on an equal footing. We apply the procedure to two types of double-dot qubits: the singlet–triplet and the semiconducting quantum dot hybrid qubit. We investigate three quantum gates that flip the qubit state: a DC pulsed gate, an AC gate based on logical qubit resonance, and a gate-like process known as stimulated Raman adiabatic passage. These gates are all mediated by an exchange interaction that is controlled experimentally using the interdot tunnel coupling g and the detuning ϵ, which sets the energy difference between the dots. Our procedure has two steps. First, we optimize the gate fidelity (f) for fixed g as a function of the other control parameters; this yields an that is universal for different types of gates. Next, we identify physical constraints on the control parameters; this yields an upper bound that is specific to the qubit-gate combination. We show that similar gate fidelities should be attainable for singlet-triplet qubits in isotopically purified Si, and for hybrid qubits in natural Si. Considerably lower fidelities are obtained for GaAs devices, due to the fluctuating magnetic fields ΔB produced by nuclear spins. PMID:24255105

  2. Interfacial Dzyaloshinskii-Moriya interaction, surface anisotropy energy, and spin pumping at spin orbit coupled Ir/Co interface

    NASA Astrophysics Data System (ADS)

    Kim, Nam-Hui; Jung, Jinyong; Cho, Jaehun; Han, Dong-Soo; Yin, Yuxiang; Kim, June-Seo; Swagten, Henk J. M.; You, Chun-Yeol

    2016-04-01

    The interfacial Dzyaloshinskii-Moriya interaction (iDMI), surface anisotropy energy, and spin pumping at the Ir/Co interface are experimentally investigated by performing Brillouin light scattering. Contrary to previous reports, we suggest that the sign of the iDMI at the Ir/Co interface is the same as in the case of the Pt/Co interface. We also find that the magnitude of the iDMI energy density is relatively smaller than in the case of the Pt/Co interface, despite the large strong spin-orbit coupling (SOC) of Ir. The saturation magnetization and the perpendicular magnetic anisotropy (PMA) energy are significantly improved due to a strong SOC. Our findings suggest that an SOC in an Ir/Co system behaves in different ways for iDMI and PMA. Finally, we determine the spin pumping effect at the Ir/Co interface, and it increases the Gilbert damping constant from 0.012 to 0.024 for 1.5 nm-thick Co.

  3. High-pressure EPR reveals conformational equilibria and volumetric properties of spin-labeled proteins

    PubMed Central

    McCoy, John; Hubbell, Wayne L.

    2011-01-01

    Identifying equilibrium conformational exchange and characterizing conformational substates is essential for elucidating mechanisms of function in proteins. Site-directed spin labeling has previously been employed to detect conformational changes triggered by some event, but verifying conformational exchange at equilibrium is more challenging. Conformational exchange (microsecond–millisecond) is slow on the EPR time scale, and this proves to be an advantage in directly revealing the presence of multiple substates as distinguishable components in the EPR spectrum, allowing the direct determination of equilibrium constants and free energy differences. However, rotameric exchange of the spin label side chain can also give rise to multiple components in the EPR spectrum. Using spin-labeled mutants of T4 lysozyme, it is shown that high-pressure EPR can be used to: (i) demonstrate equilibrium between spectrally resolved states, (ii) aid in distinguishing conformational from rotameric exchange as the origin of the resolved states, and (iii) determine the relative partial molar volume () and isothermal compressibility () of conformational substates in two-component equilibria from the pressure dependence of the equilibrium constant. These volumetric properties provide insight into the structure of the substates. Finally, the pressure dependence of internal side-chain motion is interpreted in terms of volume fluctuations on the nanosecond time scale, the magnitude of which may reflect local backbone flexibility. PMID:21205903

  4. Progress in Neutron Scattering Studies of Spin Excitations in High-T(c) Cuprates

    SciTech Connect

    Fujita M.; Tranquada J.; Hiraka, H.; Matsuda, M.; Matsuura, M.; Wakimoto, S.; Xu, G.; Yamada, K.

    2012-01-01

    Neutron scattering experiments continue to improve our knowledge of spin fluctuations in layered cuprates, excitations that are symptomatic of the electronic correlations underlying high-temperature superconductivity. Time-of-flight spectrometers, together with new and varied single crystal samples, have provided a more complete characterization of the magnetic energy spectrum and its variation with carrier concentration. While the spin excitations appear anomalous in comparison with simple model systems, there is clear consistency among a variety of cuprate families. Focusing initially on hole-doped systems, we review the nature of the magnetic spectrum, and variations in magnetic spectral weight with doping. We consider connections with the phenomena of charge and spin stripe order, and the potential generality of such correlations as suggested by studies of magnetic-field and impurity induced order. We contrast the behavior of the hole-doped systems with the trends found in the electron-doped superconductors. Returning to hole-doped cuprates, studies of translation-symmetry-preserving magnetic order are discussed, along with efforts to explore new systems. We conclude with a discussion of future challenges.

  5. High energy particle astronomy.

    NASA Technical Reports Server (NTRS)

    Buffington, A.; Muller, R. A.; Smith, L. H.; Smoot, G. F.

    1972-01-01

    Discussion of techniques currently used in high energy particle astronomy for measuring charged and neutral cosmic rays and their isotope and momentum distribution. Derived from methods developed for accelerator experiments in particle physics, these techniques help perform important particle astronomy experiments pertaining to nuclear cosmic ray and gamma ray research, electron and position probes, and antimatter searches.

  6. High Energy Astronomy Observatory

    NASA Technical Reports Server (NTRS)

    1980-01-01

    An overview of the High Energy Astronomy Observatory 2 contributions to X-ray astronomy is presented along with a brief description of the satellite and onboard telescope. Observations relating to galaxies and galactic clusters, black holes, supernova remnants, quasars, and cosmology are discussed.

  7. [Spin dependent phenomena in medium energy physics]. [Syracuse Univ. , Syracuse, New York

    SciTech Connect

    Souder, P.A.

    1992-11-01

    The Syracuse University Medium Energy Physics Group was actively engaged in several research projects. A laser was used to polarize muonic atoms with the goal of measuring fundamental spin-dependent parameters in the reaction [mu][sup [minus

  8. Some observations on spin detector response during Galileo high gain antenna deployment

    NASA Technical Reports Server (NTRS)

    Peng, Chia-Yen; Smith, Kenneth S.

    1992-01-01

    This paper summarizes a dynamic analysis conducted in support of the investigation of the anomalous deployment of the Galileo High Gain Antenna on April 11, 1991. The work was focused on modeling the spacecraft spin dynamics to predict and compare the spin detector telemetry during the antenna deployment for possible cause scenarios. The effects of analog and digital low-pass filtering, digitization, and telemetry on the reported spin rate were studied as well. The high frequency phenomena in the spin detector response are masked by the filtering and sampling of the telemetry data. However, the observed spin detector telemetery is consistent with a single rib popping free, and is most likely associated with a rib near the spin detector, or 180 deg opposite.

  9. Black hole monster in a spin releases energy!

    NASA Astrophysics Data System (ADS)

    2001-11-01

    the black hole itself is rotating. According to the team, one model fits the XMM-Newton data well. It corresponds to a theory proposed over 25 years ago by two Cambridge University astronomers. Roger Blandford and Roman Znajek had suggested that rotational energy could escape from a black hole when it is in a strong magnetic field which exerts a braking effect. This theory fits the physical laws of thermodynamics which state that energy released should be absorbed by the surrounding gas. "We have probably seen this electric dynamo effect for the very first time. Energy is being extracted from the black hole's spin and is conveyed into the innermost parts of the accretion disc, making it hotter and brighter in X-rays," says Jörn Wilms. Co-investigator Dr. Christopher Reynolds at the University of Maryland and other American members of the team contributed greatly to the theoretical interpretation of the data. "Never before have we seen energy extracted from black holes. We always see energy going in, not out," says Reynolds, who performed much of the analysis whilst at the University of Colorado. Other scientists involved in this work are James Reeves of Leicester University, United Kingdom, and Silvano Molendi of the Instituto di Fisica Cosmica "G. Occhialini", Milan, Italy. The team's conclusion that a magnetodynamic process is involved is already provoking intense debate. "We recognise that more observations are required to confirm our work," says Jörn Wilms. "But there is no disputing the presence of this exceptionally strong iron line in the spectrum of MCG-6-30-15. It is extremely puzzling and an explanation must be found." One thing is sure: only a couple of years ago, before operations with the European X-ray observatory began, no one would have dared propose such interpretations. Sufficiently detailed spectra of the kind today provided by XMM-Newton were just not available. REFERENCE "XMM-EPIC observation of MCG-6-30-15: Direct evidence for the extraction of

  10. Perpendicular spin transfer torque magnetic random access memories with high spin torque efficiency and thermal stability for embedded applications (invited)

    NASA Astrophysics Data System (ADS)

    Thomas, Luc; Jan, Guenole; Zhu, Jian; Liu, Huanlong; Lee, Yuan-Jen; Le, Son; Tong, Ru-Ying; Pi, Keyu; Wang, Yu-Jen; Shen, Dongna; He, Renren; Haq, Jesmin; Teng, Jeffrey; Lam, Vinh; Huang, Kenlin; Zhong, Tom; Torng, Terry; Wang, Po-Kang

    2014-05-01

    Magnetic random access memories based on the spin transfer torque phenomenon (STT-MRAMs) have become one of the leading candidates for next generation memory applications. Among the many attractive features of this technology are its potential for high speed and endurance, read signal margin, low power consumption, scalability, and non-volatility. In this paper, we discuss our recent results on perpendicular STT-MRAM stack designs that show STT efficiency higher than 5 kBT/μA, energy barriers higher than 100 kBT at room temperature for sub-40 nm diameter devices, and tunnel magnetoresistance higher than 150%. We use both single device data and results from 8 Mb array to demonstrate data retention sufficient for automotive applications. Moreover, we also demonstrate for the first time thermal stability up to 400 °C exceeding the requirement of Si CMOS back-end processing, thus opening the realm of non-volatile embedded memory to STT-MRAM technology.

  11. Perpendicular spin transfer torque magnetic random access memories with high spin torque efficiency and thermal stability for embedded applications (invited)

    SciTech Connect

    Thomas, Luc Jan, Guenole; Zhu, Jian; Liu, Huanlong; Lee, Yuan-Jen; Le, Son; Tong, Ru-Ying; Pi, Keyu; Wang, Yu-Jen; Shen, Dongna; He, Renren; Haq, Jesmin; Teng, Jeffrey; Lam, Vinh; Huang, Kenlin; Zhong, Tom; Torng, Terry; Wang, Po-Kang

    2014-05-07

    Magnetic random access memories based on the spin transfer torque phenomenon (STT-MRAMs) have become one of the leading candidates for next generation memory applications. Among the many attractive features of this technology are its potential for high speed and endurance, read signal margin, low power consumption, scalability, and non-volatility. In this paper, we discuss our recent results on perpendicular STT-MRAM stack designs that show STT efficiency higher than 5 k{sub B}T/μA, energy barriers higher than 100 k{sub B}T at room temperature for sub-40 nm diameter devices, and tunnel magnetoresistance higher than 150%. We use both single device data and results from 8 Mb array to demonstrate data retention sufficient for automotive applications. Moreover, we also demonstrate for the first time thermal stability up to 400 °C exceeding the requirement of Si CMOS back-end processing, thus opening the realm of non-volatile embedded memory to STT-MRAM technology.

  12. Spin polarized energy-resolved photoemission from Ni(111) using synchrotron radiation

    NASA Astrophysics Data System (ADS)

    Gudat, W.; Kisker, E.; Kuhlmann, E.; Campagna, M.

    1981-03-01

    We report on the first energy-resolved (retarding field mode) spin polarized photoemission measurement from a Ni(111) single crystal using synchrotron radiation from the ACO storage ring at LURE(ORSAY) It is shown that exchange effects can be detected for electron states well below the Fermi energy and that spin polarized, constant-initial-state spectroscopy of ferromagnets using synchrotron radiation is feasible.

  13. Observation of high-spin states in the N=84 nucleus 152Er and comparison with shell-model calculations

    NASA Astrophysics Data System (ADS)

    Kuhnert, A.; Alber, D.; Grawe, H.; Kluge, H.; Maier, K. H.; Reviol, W.; Sun, X.; Beck, E. M.; Byrne, A. P.; Hübel, H.; Bacelar, J. C.; Deleplanque, M. A.; Diamond, R. M.; Stephens, F. S.

    1992-08-01

    High-spin states in 152Er have been populated through the 116Sn(40Ar,4n)152Er reaction. Prompt and delayed γ-γ-γ-t and γ-e-t coincidences have been measured. Levels and transitions are assigned up to an excitation energy of 15 MeV and spin and parities up to 28+ at 9.7 MeV. A new isomer [t1/2=11(1) ns] has been observed at 13.4 MeV. The results are discussed in comparison with neighboring nuclei and with shell-model calculations.

  14. Yaw and spin effects on high intensity sound generation and on drag of training projectiles with ring cavities

    NASA Technical Reports Server (NTRS)

    Parthasarathy, S. P.; Cho, Y. I.; Kwack, E. Y.; Back, L. H.

    1986-01-01

    Projectiles containing axisymmetric ring cavities constitute aeroacoustic sources. These produce high intensity tones which are used for coding in the SAWE (Simulation of Area Weapons Effects) system. Experimental data obtained in a free jet facility are presented describing the effects of yaw, spin and geometric projectile parameters on sound pressure and drag. In general, the sound pressure decreases with increasing yaw angle whereas the drag increases. Spin tends to increase sound pressure levels because of a reduction in asymmetry of flow. Drag increases at zero yaw approximately as the 1.5 power of sound wavelength. A significant part of the drag increase appears to be due to energy loss by sound radiation.

  15. New high spin isomers obtained in thermal fission

    SciTech Connect

    Fogelberg, B.; Mach, H.; Gausemel, H.; Omtvedt, J. P.; Mezilev, K. A.

    1998-10-26

    The product nuclei following fission often are initially highly excited and have high angular momenta. As a consequence, there is a substantial probability for the population of isomeric yrast traps in the vicinity of closed shells. The excitation energies and decay properties of such isomers give important formation regarding the shell structure and interaction energies. Recent experiments at the OSIRIS mass separator have revealed a number of isomers in the {sup 132}Sn region having angular momenta exceeding 10 units. A brief presentation is given of some experimental results and their interpretation.

  16. Theoretical High Energy Physics

    SciTech Connect

    Christ, Norman H.; Weinberg, Erick J.

    2014-07-14

    we provide reports from each of the six faculty supported by the Department of Energy High Energy Physics Theory grant at Columbia University. Each is followed by a bibliography of the references cited. A complete list of all of the publications in the 12/1/2010-04/30/2014 period resulting from research supported by this grant is provided in the following section. The final section lists the Ph.D. dissertations based on research supported by the grant that were submitted during this period.

  17. Energy-delay performance of giant spin Hall effect switching for dense magnetic memory

    NASA Astrophysics Data System (ADS)

    Manipatruni, Sasikanth; Nikonov, Dmitri E.; Young, Ian A.

    2014-10-01

    We show that the giant spin Hall effect (GSHE) magnetoresistive random access memory (MRAM) can enable better energy delay and voltage performance than MTJ spin torque devices at 10-30 nm scaled nanomagnet dimensions. We propose a dense bit cell composed of a folded electrode to enable scaling to sub-10 nm CMOS. We derive the energy-delay trajectory and energy-delay product of GSHE and MTJ devices with an energy minimum at the magnetic characteristic time. Optimized GSHE devices with PMA can enable low voltage (<0.1 V), scaled dimensions, and fast switching time (100 ps) at an average switching energy approaching 100 aJ/bit.

  18. High temperature spin dynamics in linear magnetic chains, molecular rings, and segments by nuclear magnetic resonance

    SciTech Connect

    Adelnia, Fatemeh; Lascialfari, Alessandro; Mariani, Manuel; Ammannato, Luca; Caneschi, Andrea; Rovai, Donella; Winpenny, Richard; Timco, Grigore; Corti, Maurizio Borsa, Ferdinando

    2015-05-07

    We present the room temperature proton nuclear magnetic resonance (NMR) nuclear spin-lattice relaxation rate (NSLR) results in two 1D spin chains: the Heisenberg antiferromagnetic (AFM) Eu(hfac){sub 3}NITEt and the magnetically frustrated Gd(hfac){sub 3}NITEt. The NSLR as a function of external magnetic field can be interpreted very well in terms of high temperature spin dynamics dominated by a long time persistence of the decay of the two-spin correlation function due to the conservation of the total spin value for isotropic Heisenberg chains. The high temperature spin dynamics are also investigated in Heisenberg AFM molecular rings. In both Cr{sub 8} closed ring and in Cr{sub 7}Cd and Cr{sub 8}Zn open rings, i.e., model systems for a finite spin segment, an enhancement of the low frequency spectral density is found consistent with spin diffusion but the high cut-off frequency due to intermolecular anisotropic interactions prevents a detailed analysis of the spin diffusion regime.

  19. NMR Investigation of beta-Substituted High-Spin and Low-Spin Iron(III) Tetraphenylporphyrins.

    PubMed

    Wojaczynski, Jacek; Latos-Grazynski, Lechoslaw; Hrycyk, Witold; Pacholska, Ewa; Rachlewicz, Krystyna; Szterenberg, Ludmila

    1996-11-01

    The NMR spectra of a series of beta-substituted iron(III) tetraphenylporphyrin (2-X-TPP) complexes have been studied to elucidate the relationship between the electron donating/withdrawing properties of the 2-substituent and the (1)H NMR spectral pattern. The electronic nature of the substituent has been significantly varied and covered the -0.6 to 0.8 Hammett constant range. Both high-spin and low-spin complexes of the general formula (2-X-TPP)Fe(III)Cl and [(2-X-TPP)Fe(III)(CN)(2)](-) have been investigated. The (1)H NMR data for the following substituents (X) have been reported: py(+), NO(2), CN, CH(3), BzO (C(6)H(5)COO), H, D, Br, Cl, CH(3), NH(2), NH(3)(+), NHCH(3), OH, and O(-). The (1)H NMR resonances for low-spin dicyano complexes have been completely assigned by a combination of two-dimensional COSY and NOESY experiments. In the case of selected high-spin complexes, the 3-H resonance has been identified by the selective deuteration of all but the 3-H position. The pattern of unambiguously assigned seven pyrrole resonances reflects the asymmetry imposed by 2-substitution and has been used as an unique (1)H NMR spectroscopic probe to map the spin density distribution. The pyrrole isotropic shifts of [(2-X-TPP)Fe(III)(CN)(2)](-) are dominated by the contact term. In order to quantify the substituent effect, the dependence of isotropic shift of all low-spin pyrrole resonances and 3-H high-spin pyrrole resonance versus Hammett constants has been studied. The electronic effect is strongly localized at the beta-substituted pyrrole. The major change of the isotropic shift has also been noted for only one of two adjacent pyrrole rings, i.e., at 7-H and 8-H positions. These neighboring protons, located on a single pyrrole ring, experienced opposite shift changes when electron withdrawing/donating properties were modified. Two other pyrrole rings for all investigated derivatives revealed considerably smaller, substituent related, isotropic shift changes. A long

  20. Direct observation of a highly spin-polarized organic spinterface at room temperature

    PubMed Central

    Djeghloul, F.; Ibrahim, F.; Cantoni, M.; Bowen, M.; Joly, L.; Boukari, S.; Ohresser, P.; Bertran, F.; Le Fèvre, P.; Thakur, P.; Scheurer, F.; Miyamachi, T.; Mattana, R.; Seneor, P.; Jaafar, A.; Rinaldi, C.; Javaid, S.; Arabski, J.; Kappler, J. -P; Wulfhekel, W.; Brookes, N. B.; Bertacco, R.; Taleb-Ibrahimi, A.; Alouani, M.; Beaurepaire, E.; Weber, W.

    2013-01-01

    Organic semiconductors constitute promising candidates toward large-scale electronic circuits that are entirely spintronics-driven. Toward this goal, tunneling magnetoresistance values above 300% at low temperature suggested the presence of highly spin-polarized device interfaces. However, such spinterfaces have not been observed directly, let alone at room temperature. Thanks to experiments and theory on the model spinterface between phthalocyanine molecules and a Co single crystal surface, we clearly evidence a highly efficient spinterface. Spin-polarised direct and inverse photoemission experiments reveal a high degree of spin polarisation at room temperature at this interface. We measured a magnetic moment on the molecule's nitrogen π orbitals, which substantiates an ab-initio theoretical description of highly spin-polarised charge conduction across the interface due to differing spinterface formation mechanisms in each spin channel. We propose, through this example, a recipe to engineer simple organic-inorganic interfaces with remarkable spintronic properties that can endure well above room temperature. PMID:23412079

  1. High-resolution NMR of anisotropic samples with spinning away from the magic angle

    SciTech Connect

    Sakellariou, Dimitris; Meriles, Carlos A.; Martin, Rachel W.; Pines, Alexander

    2003-03-31

    High-resolution NMR of samples in the solid state is typically performed under mechanical sample spinning around an axis that makes an angle, called the magic angle, of 54.7 degrees with the static magnetic field. There are many cases in which geometrical and engineering constraints prevent spinning at this specific angle. Implementations of in-situ and ex-situ magic angle field spinning might be extremely demanding because of the power requirements or an inconvenient sample size or geometry. Here we present a methodology based on switched angle spinning between two angles, none of which is the magic angle, which provide both isotropic and anisotropic information. Using this method, named Projected Magic Angle Spinning, we were able to obtain resolved isotropic chemical shifts in spinning samples where the broadening is mostly inhomogeneous.

  2. Isospin Symmetry at High Spin Studied via Nucleon Knockout from Isomeric States

    NASA Astrophysics Data System (ADS)

    Milne, S. A.; Bentley, M. A.; Simpson, E. C.; Baugher, T.; Bazin, D.; Berryman, J. S.; Bruce, A. M.; Davies, P. J.; Diget, C. Aa.; Gade, A.; Henry, T. W.; Iwasaki, H.; Lemasson, A.; Lenzi, S. M.; McDaniel, S.; Napoli, D. R.; Nichols, A. J.; Ratkiewicz, A.; Scruton, L.; Stroberg, S. R.; Tostevin, J. A.; Weisshaar, D.; Wimmer, K.; Winkler, R.

    2016-08-01

    One-neutron knockout reactions have been performed on a beam of radioactive 53Co in a high-spin isomeric state. The analysis is shown to yield a highly selective population of high-spin states in an exotic nucleus with a significant cross section, and hence represents a technique that is applicable to the planned new generation of fragmentation-based radioactive beam facilities. Additionally, the relative cross sections among the excited states can be predicted to a high level of accuracy when reliable shell-model input is available. The work has resulted in a new level scheme, up to the 1 1+ band-termination state, of the proton-rich nucleus 52Co (Z =27 , N =25 ). This has in turn enabled a study of mirror energy differences in the A =52 odd-odd mirror nuclei, interpreted in terms of isospin-nonconserving (INC) forces in nuclei. The analysis demonstrates the importance of using a full set of J -dependent INC terms to explain the experimental observations.

  3. Isospin Symmetry at High Spin Studied via Nucleon Knockout from Isomeric States.

    PubMed

    Milne, S A; Bentley, M A; Simpson, E C; Baugher, T; Bazin, D; Berryman, J S; Bruce, A M; Davies, P J; Diget, C Aa; Gade, A; Henry, T W; Iwasaki, H; Lemasson, A; Lenzi, S M; McDaniel, S; Napoli, D R; Nichols, A J; Ratkiewicz, A; Scruton, L; Stroberg, S R; Tostevin, J A; Weisshaar, D; Wimmer, K; Winkler, R

    2016-08-19

    One-neutron knockout reactions have been performed on a beam of radioactive ^{53}Co in a high-spin isomeric state. The analysis is shown to yield a highly selective population of high-spin states in an exotic nucleus with a significant cross section, and hence represents a technique that is applicable to the planned new generation of fragmentation-based radioactive beam facilities. Additionally, the relative cross sections among the excited states can be predicted to a high level of accuracy when reliable shell-model input is available. The work has resulted in a new level scheme, up to the 11^{+} band-termination state, of the proton-rich nucleus ^{52}Co (Z=27, N=25). This has in turn enabled a study of mirror energy differences in the A=52 odd-odd mirror nuclei, interpreted in terms of isospin-nonconserving (INC) forces in nuclei. The analysis demonstrates the importance of using a full set of J-dependent INC terms to explain the experimental observations. PMID:27588851

  4. Spin-controlled orbital motion in tightly focused high-order Laguerre-Gaussian beams.

    PubMed

    Cao, Yongyin; Zhu, Tongtong; Lv, Haiyi; Ding, Weiqiang

    2016-02-22

    Spin angular momentum can contribute to both optical force and torque exerted on spheres. Orbit rate of spheres located in tightly focused LG beams with the same azimuthal mode index l is spin-controlled due to spin-orbit coupling. Laguerre-Gaussian beams with high-order azimuthal mode are used here to study the orbit rate of dielectric spheres. Orbit rates of spheres with varying sizes and refravtive indices are investigated as well as optical forces acting on spheres in LG beams with different azimuthal modes. These results would be much helpful to investigation on optical rotation and transfer of spin and orbital angular momentum. PMID:26906996

  5. Exact spin dynamics of inhomogeneous 1-d systems at high temperature

    NASA Astrophysics Data System (ADS)

    Danieli, E. P.; Pastawski, H. M.; Levstein, P. R.

    2002-07-01

    The evaluation of spin excitation dynamics in finite 1-d systems of spins {1}/{2} with XY exchange interaction J acquired new interest because NMR experiments at high temperature ( kBT≫ J) confirmed the predicted spin wave behavior of mesoscopic echoes. In this work, we use the Jordan-Wigner transformation to obtain the exact dynamics of inhomogeneous chains and rings where the evolution is reduced to one-body dynamics. For higher dimensions, the spin excitations manifest many-body effects that can be interpreted as a simple dynamics of non-interacting fermions plus a decoherent process.

  6. Phenomena at very high spins. [Approx. 70 h-bar; review

    SciTech Connect

    Stephens, F.S.

    1980-03-01

    The present talk has three parts: first, a discussion of current ideas about the physics of very high spin states; second, some comments about noncollective behavior up to the highest spins where it is known, approx. 40 h; and finally, a presentation of the newest method for studying collective behavior up to spins of 60 to 70 h. The intention is that the overview presented in the first part will be sufficiently broad to indicate the relationship of the noncollective and collective behavior discussed in the other parts, and to provide some understanding of the compromise in behavior that seems to occur at the very highest spins. 13 figures.

  7. High energy from space

    NASA Technical Reports Server (NTRS)

    Margon, Bruce; Canizares, Claude; Catura, Richard C.; Clark, George W.; Fichtel, Carl E.; Friedman, Herbert; Giacconi, Riccardo; Grindlay, Jonathan E.; Helfand, David J.; Holt, Stephen S.

    1991-01-01

    The following subject areas are covered: (1) important scientific problems for high energy astrophysics (stellar activity, the interstellar medium in galaxies, supernovae and endpoints of stellar evolution, nucleosynthesis, relativistic plasmas and matter under extreme conditions, nature of gamma-bursts, identification of black holes, active nuclei, accretion physics, large-scale structures, intracluster medium, nature of dark matter, and the X- and gamma-ray background); (2) the existing experimental programs (Advanced X-Ray Astrophysics Facility (AXAF), Gamma Ray Observatory (GRO), X-Ray Timing Explorer (XTE), High Energy Transient Experiment (HETE), U.S. participation in foreign missions, and attached Shuttle and Space Station Freedom payloads); (3) major missions for the 1990's; (4) a new program of moderate missions; (5) new opportunities for small missions; (6) technology development issues; and (7) policy issues.

  8. High energy transients

    NASA Technical Reports Server (NTRS)

    Woosley, S. E.

    1984-01-01

    A meeting was convened on the campus of the University of California at Santa Cruz during the two-week interval July 11 through July 22, 1983. Roughly 100 participants were chosen so as to give broad representation to all aspects of high energy transients. Ten morning review sessions were held in which invited speakers discussed the current status of observations and theory of the above subjects. Afternoon workshops were also held, usually more than one per day, to informally review various technical aspects of transients, confront shortcomings in theoretical models, and to propose productive courses for future research. Special attention was also given to the instrumentation used to study high energy transient and the characteristics and goals of a dedicated space mission to study transients in the next decade were determined. A listing of articles written by various members of the workshop is included.

  9. Mildly Recycled Pulsars at High-Energies

    NASA Astrophysics Data System (ADS)

    Pellizzoni, A.

    2011-08-01

    Mildly recyled pulsars (MRP), conventionally defined as neutron star having spin period in the 20-100 ms range and surface magnetic field <1011 Gauss, probably rise from binary systems (disrupted or not) with an intermediate or an high mass companion. Despite their relatively low spin-down energies compared to the ``fully'' recycled millisecond pulsars (arising from common low mass X-ray binaries), nearby MRPs can be detected by deep X-ray observations and by timing analysis of the very long data span provided by gamma-ray space detectors. The discovery of peculiar timing and spectral properties, possibly transitional, of the MRPs can be of the utmost importance to link different classes of neutron stars and study their evolution.

  10. Non-additive three-body interaction energies for H3 (quartet spin state)

    NASA Astrophysics Data System (ADS)

    Zhang, Z. C.; Allnatt, A. R.; Talman, James D.; Meath, William J.

    The results of an Unsold average energy calculation of the non-additive interaction energy for H3 (quartet spin state) are presented for equilateral triangular configurations. They are discussed in the context of the problems associated with the representation of non-additive energies for the interaction of closed-shell species.

  11. High Energy Density Microwaves

    SciTech Connect

    Phillips, R.M.

    1999-04-01

    These proceedings represent papers presented at the RF98 Workshop entitled `High Energy Density Microwaves` held in California in October, 1998. The topics discussed were predominantly accelerator{minus}related. The Workshop dealt, for the most part, with the generation and control of electron beams, the amplification of RF signals, the design of mode converters, and the effect of very high RF field gradients. This Workshop was designed to address the concerns of the microwave tube industry worldwide, the plasma physicists who deal with very high beam currents and gigawatts of RF power, and researchers in accelerator centers around the world. Papers were presented on multibeam klystrons, gyrotron development, plasmas in microwave tubes, RF breakdown, and alternatives to conventional linear coliders at 1 TeV and above. The Workshop was partially sponsored by the US Department of Energy. There were 46 papers presented at the conference,out of which 19 have been abstracted for the Energy,Science and Technology database.(AIP)

  12. Spin currents injected electrically and thermally from highly spin polarized Co{sub 2}MnSi

    SciTech Connect

    Pfeiffer, Alexander; Reeve, Robert M.; Kronenberg, Alexander; Jourdan, Martin; Kläui, Mathias; Hu, Shaojie; Kimura, Takashi

    2015-08-24

    We demonstrate the injection and detection of electrically and thermally generated spin currents probed in Co{sub 2}MnSi/Cu lateral spin valves. Devices with different electrode separations are patterned to measure the non-local signal as a function of the electrode spacing and we determine a relatively high effective spin polarization α of Co{sub 2}MnSi to be 0.63 and the spin diffusion length of Cu to be 500 nm at room temperature. The electrically generated non-local signal is measured as a function of temperature and a maximum signal is observed for a temperature of 80 K. The thermally generated non-local signal is measured as a function of current density and temperature in a second harmonic measurement detection scheme. We find different temperature dependences for the electrically and thermally generated non-local signals, which allows us to conclude that the temperature dependence of the signals is not just dominated by the transport in the Cu wire, but there is a crucial contribution from the different generation mechanisms, which has been largely disregarded till date.

  13. Nuclear shape transitions and some properties of aligned-particle configurations at high spin

    SciTech Connect

    Koo, T.L.; Chowdhury, P.; Emling, H.

    1982-01-01

    Two topics are addressed in this paper. First, we discuss the variation of shapes with spin and neutron number for nuclei in the N approx. = 88 transitional region. Second, we present comments on the feeding times of very high spin single-particle yrast states.

  14. Energy harvesting using rattleback: Theoretical analysis and simulations of spin resonance

    NASA Astrophysics Data System (ADS)

    Nanda, Aditya; Singla, Puneet; Karami, M. Amin

    2016-05-01

    This paper investigates the spin resonance of a rattleback subjected to base oscillations which is able to transduce vibrations into continuous rotary motion and, therefore, is ideal for applications in Energy harvesting and Vibration sensing. The rattleback is a toy with some curious properties. When placed on a surface with reasonable friction, the rattleback has a preferred direction of spin. If rotated anti to it, longitudinal vibrations are set up and spin direction is reversed. In this paper, the dynamics of a rattleback placed on a sinusoidally vibrating platform are simulated. We can expect base vibrations to excite the pitch motion of the rattleback, which, because of the coupling between pitch and spin motion, should cause the rattleback to spin. Results are presented which show that this indeed is the case-the rattleback has a mono-peak spin resonance with respect to base vibrations. The dynamic response of the rattleback was found to be composed of two principal frequencies that appeared in the pitch and rolling motions. One of the frequencies was found to have a large coupling with the spin of the rattleback. Spin resonance was found to occur when the base oscillatory frequency was twice the value of the coupled frequency. A linearized model is developed which can predict the values of the two frequencies accurately and analytical expressions for the same in terms of the parameters of the rattleback have been derived. The analysis, thus, forms an effective and easy method for obtaining the spin resonant frequency of a given rattleback. Novel ideas for applications utilizing the phenomenon of spin resonance, for example, an energy harvester composed of a magnetized rattleback surrounded by ferromagnetic walls and a small scale vibration sensor comprising an array of several magnetized rattlebacks, are included.

  15. Photon strength functions in 177Lu: Study of scissors resonance in high-spin region

    NASA Astrophysics Data System (ADS)

    Bečvář, F.; Krtička, M.; Tomandl, I.; Valenta, S.

    2015-05-01

    The nucleus 177Lu is characteristic by an unusually high value of the thermal-neutron capturing state spin, J = 13/2, and by distinct low-energy rotational bands built on the 7/2+ ground state and the 9/2- level at 150 keV. The γ cascades connecting the capturing state with the members of these bands carry unique information about the role of identical M1 scissors-mode resonances, built according to Brink hypothesis assumingly on each energy level, even in conditions of fast nuclear rotation. With this motivation we measured a set of spectra of two-step γ cascades following the thermal neutron capture in 176Lu. The measurement was performed at neutron beam of the LWR-15 Reactor in Řež. From the analysis of these spectra the common parameters of the scissors resonances were deduced. The obtained results are discussed.

  16. Spin correlations in electron-doped high-Tc superconductor

    NASA Astrophysics Data System (ADS)

    Fujita, M.

    2007-11-01

    Spin correlations in the electron-doped Pr1-xLaCexCuO4 have been investigated by neutron-scattering and muon rotation/relaxation measurements. The low-enegy spin correlations were found to be in commensurate with the wide superconducting phase, unlike the incommensurate ones in the hole-doped La2-xSrxCuO4. No enhancement of the magnetic order by impurity-doping and applying magnetic fields was observed, although the superconductivity is effectively suppressed, compared to that in the hole-doped system. Distinct impurity and magnetic field effects between the static spin correlation in the electron-doped system and those in the hole-doped systems suggest the different magnetic ground state in the two systems.

  17. High spin polarization and the origin of unique ferromagnetic ground state in CuFeSb

    NASA Astrophysics Data System (ADS)

    Sirohi, Anshu; Singh, Chandan K.; Thakur, Gohil S.; Saha, Preetha; Gayen, Sirshendu; Gaurav, Abhishek; Jyotsna, Shubhra; Haque, Zeba; Gupta, L. C.; Kabir, Mukul; Ganguli, Ashok K.; Sheet, Goutam

    2016-06-01

    CuFeSb is isostructural to the ferro-pnictide and chalcogenide superconductors and it is one of the few materials in the family that are known to stabilize in a ferromagnetic ground state. Majority of the members of this family are either superconductors or antiferromagnets. Therefore, CuFeSb may be used as an ideal source of spin polarized current in spin-transport devices involving pnictide and the chalcogenide superconductors. However, for that the Fermi surface of CuFeSb needs to be sufficiently spin polarized. In this paper we report direct measurement of transport spin polarization in CuFeSb by spin-resolved Andreev reflection spectroscopy. From a number of measurements using multiple superconducting tips we found that the intrinsic transport spin polarization in CuFeSb is high (˜47%). In order to understand the unique ground state of CuFeSb and the origin of large spin polarization at the Fermi level, we have evaluated the spin-polarized band structure of CuFeSb through first principles calculations. Apart from supporting the observed 47% transport spin polarization, such calculations also indicate that the Sb-Fe-Sb angles and the height of Sb from the Fe plane are strikingly different for CuFeSb than the equivalent parameters in other members of the same family thereby explaining the origin of the unique ground state of CuFeSb.

  18. Spectroscopy and high-spin structure of 210Fr: Isomerism and potential evidence for configuration mixing

    NASA Astrophysics Data System (ADS)

    Margerin, V.; Lane, G. J.; Dracoulis, G. D.; Palalani, N.; Smith, M. L.; Stuchbery, A. E.

    2016-06-01

    The structure of 210Fr has been established up to an excitation energy of ˜5.5 MeV and spins of ˜25 ℏ , via time-correlated γ -ray spectroscopy and using the 197Au(18O,5 n )210Fr reaction with pulsed beams at an energy of 97 MeV. A significantly different level scheme has been obtained compared to previous publications. Several isomers are reported here, including a Jπ=(23) +,τ =686 (9 ) -ns state at 4417 keV and a 10-, 29.8(11)-ns state at 1113 keV. The former isomer has been associated with the π (h9/2 3i13/2 2) ν (p1/2 -2f5/2 -1) configuration and decays via proposed E 3 transitions with strengths of 8.4(3) and 21.2(8) W.u. There are only very few known cases of a high-spin isomer decaying via two parallel E 3 transitions. Indeed, this is not seen in other Fr nuclei, and consequently these strengths differ from related decays in the neighboring isotopes. However, by examining the systematics of E 3 transitions in trans-lead nuclei, we suggest that the weaker of the two transitions decays to a mixed 20- state. Systematics of the 10- isomer are also discussed. Comparisons are made between the observed spectrum of states and those predicted from semiempirical shell-model calculations.

  19. Neutron scattering studies of spin-phonon hybridization and superconducting spin gaps in the high-temperature superconductor La2-x(Sr,Ba)xCuO4

    NASA Astrophysics Data System (ADS)

    Wagman, J. J.; Carlo, J. P.; Gaudet, J.; Van Gastel, G.; Abernathy, D. L.; Stone, M. B.; Granroth, G. E.; Kolesnikov, A. I.; Savici, A. T.; Kim, Y. J.; Zhang, H.; Ellis, D.; Zhao, Y.; Clark, L.; Kallin, A. B.; Mazurek, E.; Dabkowska, H. A.; Gaulin, B. D.

    2016-03-01

    We present time-of-flight neutron scattering measurements on single crystals of La2-xBaxCuO4 (LBCO) with 0 ≤x ≤0.095 and La2-xSrxCuO4 (LSCO) with x =0.08 and 0.11. This range of dopings spans much of the phase diagram relevant to high-temperature cuprate superconductivity, ranging from insulating, three-dimensional commensurate long-range antiferromagnetic order, for x ≤0.02 , to two-dimensional (2D) incommensurate antiferromagnetism coexisting with superconductivity for x ≥0.05 . Previous work on lightly doped LBCO with x =0.035 showed a clear enhancement of the inelastic scattering coincident with the low-energy crossings of the highly dispersive spin excitations and quasi-2D optic phonons. The present work extends these measurements across the phase diagram and shows this enhancement to be a common feature to this family of layered quantum magnets. Furthermore, we show that the low-temperature, low-energy magnetic spectral weight is substantially larger for samples with nonsuperconducting ground states relative to any of the samples with superconducting ground states. Spin gaps, suppression of low-energy magnetic spectral weight as a function of decreasing temperature, are observed in both superconducting LBCO and LSCO samples, consistent with previous observations for superconducting LSCO.

  20. Neutron scattering studies of spin-phonon hybridization and superconducting spin gaps in the high temperature superconductor La2-x(Sr;Ba)xCuO4

    DOE PAGESBeta

    Wagman, J. J.; Carlo, Jeremy P.; Gaudet, J.; Van Gastel, G. J.; Abernathy, Douglas L.; Stone, Matthew B.; Granroth, Garrett E.; Kolesnikov, Alexander I.; Savici, Andrei T.; Kim, Young -June; et al

    2016-03-14

    We present time-of-flight neutron-scattering measurements on single crystals of La2-xBaxCuO4 (LBCO) with 0 ≤ x ≤ 0.095 and La2-xSrxCuO4 (LSCO) with x = 0.08 and 0.11. This range of dopings spans much of the phase diagram relevant to high temperature cuprate superconductivity, ranging from insulating, three dimensional commensurate long range antiferromagnetic order for x ≤ 0.02 to two dimensional (2D) incommensurate antiferromagnetism co-existing with superconductivity for x ≥ 0.05. Previous work on lightly doped LBCO with x = 0.035 showed a clear resonant enhancement of the inelastic scattering coincident with the low energy crossings of the highly dispersive spin excitationsmore » and quasi-2D optic phonons. The present work extends these measurements across the phase diagram and shows this enhancement to be a common feature to this family of layered quantum magnets. Furthermore we show that the low temperature, low energy magnetic spectral weight is substantially larger for samples with non-superconducting ground states relative to any of the samples with superconducting ground states. Lastly spin gaps, suppression of low energy magnetic spectral weight, are observed in both superconducting LBCO and LSCO samples, consistent with previous observations for superconducting LSCO« less

  1. On numerical nonlinear analysis of highly flexible spinning cantilevers

    NASA Technical Reports Server (NTRS)

    Utku, S.; El-Essawi, M.; Salama, M.

    1981-01-01

    The general nonlinear discretized equations of motion of spinning elastic solids and structures are derived as a set of nonlinear ordinary differential equations for the case when the strain-displacement and velocity-displacement relations are nonlinear up to the second order. It is shown that the cost of generation of such equations is proportional to the fourth power of the number of degrees of freedom. A computer program is written to automatically generate the equations for the case of spinning cantilevers with initial imperfections. The types and the number of the coordinate functions used in the trial solution are parameters of the program.

  2. The free energy in a class of quantum spin systems and interchange processes

    NASA Astrophysics Data System (ADS)

    Björnberg, J. E.

    2016-07-01

    We study a class of quantum spin systems in the mean-field setting of the complete graph. For spin S = 1/2, the model is the Heisenberg ferromagnet, and for general spin S ∈ 1/2 N, it has a probabilistic representation as a cycle-weighted interchange process. We determine the free energy and the critical temperature (recovering results by Tóth and by Penrose when S = 1/2). The critical temperature is shown to coincide (as a function of S) with that of the q = 2S + 1 state classical Potts model, and the phase transition is discontinuous when S ≥ 1.

  3. Mapping between the Heisenberg XX Spin Chain and Low-Energy QCD

    NASA Astrophysics Data System (ADS)

    Pérez-García, David; Tierz, Miguel

    2014-04-01

    By using random matrix models, we uncover a connection between the low-energy sector of four-dimensional QCD at finite volume and the Heisenberg XX model in a 1D spin chain. This connection allows us to relate crucial properties of QCD with physically meaningful properties of the spin chain, establishing a dictionary between both worlds. For the spin chain, we predict a third-order phase transition and a Tracy-Widom law in the transition region. We also comment on possible numerical implications of the connection as well as on possible experimental implementations.

  4. Spin rotators and split Siberian Snakes

    SciTech Connect

    Roser, Thomas

    1994-03-01

    The study of spin effects in the collision of polarized high energy beams requires flexible and compact spin rotators to manipulate the beam polarization direction. Design criteria and specific examples are presented for high energy, orbit transparent spin rotators ranging from small angle rotators to be used for the excitation of spin resonances to large angle rotators to be used as Siberian Snakes. It is shown that all the requirements for spin rotators can be met with a simple 6-magnet spin rotator design, for which a complete continuous solution is presented.

  5. Theoretical studies of possible toroidal high-spin isomers in the light-mass region

    DOE PAGESBeta

    Staszczak, A.; Wong, Cheuk-Yin

    2016-05-11

    We review our theoretical knowledge of possible toroidal high-spin isomers in the light mass region in 28 A 52 obtained previously in cranked Skyrme-Hartree-Fock calculations. We report additional toroidal high-spin isomers in 56Ni with I=114 and 140, which follow the same (multi-particle) (multi-hole) systematics as other toroidal high-spin isomers. We examine the production of these exotic nuclei by fusion of various projectiles on 20Ne or 28Si as an active target in time-projection-chamber (TPC) experiments.

  6. Theoretical studies of possible toroidal high-spin isomers in the light-mass region

    NASA Astrophysics Data System (ADS)

    Staszczak, Andrzej; Wong, Cheuk-Yin

    2016-05-01

    We review our theoretical knowledge of possible toroidal high-spin isomers in the light mass region in 28≤A≤52 obtained previously in cranked Skyrme-Hartree-Fock calculations. We report additional toroidal high-spin isomers in 56Ni with I=114ħ and 140ħ, which follow the same (multi-particle)-(multi-hole) systematics as other toroidal high-spin isomers. We examine the production of these exotic nuclei by fusion of various projectiles on 20Ne or 28Si as an active target in time-projection-chamber (TPC) experiments.

  7. Time-resolved and energy-dispersed spin excitation in ferromagnets and clusters under influence of femtosecond laser pulses

    NASA Astrophysics Data System (ADS)

    Hartenstein, T.; Lefkidis, G.; Hübner, W.; Zhang, G. P.; Bai, Y.

    2009-04-01

    When an ultrafast laser impinges a magnetic material, it excites charge and then, via spin-orbit-coupling, spin. This holds great promise for the future magnetic storage. However, the coupling of the two dynamics is far from clear, which hampers the experimental effort in femtosecond magnetism. Since not every excitation induces the same spin excitation, a clear understanding of the correlation between charge and spin is crucial. In this paper we investigate in a complete first-principles manner the energy dispersion of the spin-moment change in ferromagnetic Ni and the effect of the distance between the magnetic centers upon the spin localization and local-spin-flip times in metallic chains. Thus we establish the missing link between the spin-momentum change and the density-of-states change, and derive rules-of-thumb for localized spin manipulation.

  8. High-energy transients.

    PubMed

    Gehrels, Neil; Cannizzo, John K

    2013-06-13

    We present an overview of high-energy transients in astrophysics, highlighting important advances over the past 50 years. We begin with early discoveries of γ-ray transients, and then delve into physical details associated with a variety of phenomena. We discuss some of the unexpected transients found by Fermi and Swift, many of which are not easily classifiable or in some way challenge conventional wisdom. These objects are important insofar as they underscore the necessity of future, more detailed studies. PMID:23630376

  9. Very high energy colliders

    NASA Astrophysics Data System (ADS)

    Richter, B.

    1985-05-01

    The required emittance in very high energy machines are small. It will be a real challenge to produce these small emittances and to maintain them during acceleration. The small emittances probably make acceleration by laser techniques easier, if such techniques will be practical at all. The beam spot sizes are very small indeed. It will be a challenge to design beam transport systems with the necessary freedom from aberration required for these small spot sizes. It would of course help if the beta functions at the collision points could be reduced. Beam power will be large - to paraphrase the old saying, power is money - and efficient acceleration systems will be required.

  10. High energy electron cooling

    SciTech Connect

    Parkhomchuk, V.

    1997-09-01

    High energy electron cooling requires a very cold electron beam. The questions of using electron cooling with and without a magnetic field are presented for discussion at this workshop. The electron cooling method was suggested by G. Budker in the middle sixties. The original idea of the electron cooling was published in 1966. The design activities for the NAP-M project was started in November 1971 and the first run using a proton beam occurred in September 1973. The first experiment with both electron and proton beams was started in May 1974. In this experiment good result was achieved very close to theoretical prediction for a usual two component plasma heat exchange.

  11. Spin-polaron theory of high-{Tc} superconductivity: 2, electronic structure of the CuO{sub 2} planes

    SciTech Connect

    Wood, R.F.

    1993-06-01

    After an introductory discussion of electronic structure calculations for the CuO{sub 2} planes in the copper-oxide based high-{Tc} superconductors, the method suggested by Slater for studying antiferromagnetic (AF) metals is described. In this method, as applied here, the chemical unit cell is doubled to form a magnetic unit cell which contains one Cu ion with predominantly up spin and one with predominantly down spin. Down spins are kept off up-spin sites, and conversely, by the introduction of a Hubbard U term. As a result, the band structure obtained is typical of that for a Mott-Hubbard (M-H) or, more generally, a charge transfer insulator. Conductivity in the a-b plane results when holes are introduced into the M-H valence band. The band structure as a function of the parameters in Koster-Slater type calculations is discussed and the Fermi surface is described. A calculation of the delocalization energy for spin-polaron formation is carried out within the context of the band calculations.

  12. Prospects at high energies

    SciTech Connect

    Quigg, C.

    1988-11-01

    I discuss some possibilities for neutrino experiments in the fixed-target environment of the SPS, Tevatron, and UNK, with their primary proton beams of 0.4, 0.9, and 3.0 TeV. The emphasis is on unfinished business: issues that have been recognized for some time, but not yet resolved. Then I turn to prospects for proton-proton colliders to explore the 1-TeV scale. I review the motivation for new physics in the neighborhood of 1 TeV and mention some discovery possibilities for high-energy, high-luminosity hadron colliders and the implications they would have for neutrino physics. I raise the possibility of the direct study of neutrino interactions in hadron colliders. I close with a report on the status of the SSC project. 38 refs., 17 figs.

  13. Average magnetic moments of pre-yrast high spin states in {sup 166,165}Hf

    SciTech Connect

    Weissman, L.; Hass, M.; Broude, C.

    1996-01-01

    The average magnetic moments of high spin states in Hf isotopes were determined in a transient field measurement at the 14 MV Koffler accelerator of the Weizmann Institute. The reaction {sup 130}Te({sup 40}Ca,{ital xn}){sup 166,165}Hf at beam energies from 167 to 182.5 MeV was used to populate different high spin regions and provide the recoiling Hf nuclei with sufficient velocity to traverse the 2.9 mg/cm{sup 2} Gd ferromagnetic layer. Standard double ratios and angular distributions for various low level transitions were measured to determine precession angles. These carry information regarding the average {ital g} factor of unobservable transitions at medium excitation. To obtain a more quantitative analysis regarding the time-decay history of the {gamma} cascade, Monte Carlo simulations of the cascade were carried out. The significance of the results for understanding the single particle nature of these pre-yrast levels is discussed. {copyright} {ital 1996 The American Physical Society.}

  14. High-spin level structure in {sup 94,95}Mo

    SciTech Connect

    Zhang, Y. H.; Hasegawa, M.; Guo, W. T.; Liu, M. L.; Zhou, X. H.; De Angelis, G.; Axiotis, T. M.; Gadea, A.; Marginean, N.; Martinez; Napoli, D. R.; Rusu, C.; Podolyak, Zs.; Ur, C.; Bazzacco, D.; Brandolini, F.; Lunardi, S.; Lenzi, S. M.; Menegazzo, R.; Schwengner, R.

    2009-04-15

    High-spin level structures of {sup 94,95}Mo have been reinvestigated via the {sup 16}O({sup 82}Se,xn{gamma}){sup 94,95}Mo(x=4,3) reactions at E({sup 82}Se)=460 MeV. The previously reported level schemes of these two nuclei have been largely modified up to {approx}11 MeV in excitation energy due to identifications of some important linking transitions. Shell-model calculations have been made in the model space of {pi}(p{sub 1/2},g{sub 9/2},d{sub 5/2}){sup 4} and {nu}(d{sub 5/2},s{sub 1/2},d{sub 3/2},g{sub 7/2},h{sub 11/2}){sup 2(3)} and compared with the modified level schemes. The structures of the newly assigned high-spin states in {sup 94,95}Mo have been discussed.

  15. High-spin states in the five-valence-particle nucleus {sup 213}Po

    SciTech Connect

    Astier, Alain; Porquet, Marie-Genevieve

    2011-03-15

    Excited states in {sup 213}Po have been populated using the {sup 18}O+ {sup 208}Pb reaction at 85 MeV beam energy and studied with the Euroball IV {gamma} multidetector array. The level scheme has been built up to {approx}2.0 MeV excitation energy and spin I{approx}25/2({h_bar}/2{pi}) from the triple {gamma} coincidence data. Spin and parity values of several yrast states have been assigned from the {gamma} angular properties. The configurations of the yrast states are discussed using results of empirical shell-model calculations and by analogy with the neighboring nuclei. The spin and parity values of several low-spin states of {sup 213}Po previously identified from the {beta} decay of {sup 213}Bi are revised.

  16. High-spin multiplicities in ferromagnetic ground states of supramolecular halide complexes based on the gadolinium chloride

    NASA Astrophysics Data System (ADS)

    Paduani, C.

    2016-03-01

    Calculations using density functional theory are performed to study supramolecular assemblage of high spin halide complexes based on the gadolinium chloride. With the addition of Cl atoms to both Gd and B in number that exceeds their formal valence by 1 the calculated vertical detachment energy increases to 6.08 and 5.57 eV in GdCl4 and BCl4, respectively, indicating superhalogen behavior. By using BCl4 and GdCl4 clusters as building blocks to decorate the Gd atom the vertical detachment energy increases to 7.12 and 7.70 eV in the anionic clusters Gd(BCl4)4- and Gd(GdCl4)4-, respectively, which is indicative of hyperhalogen behavior. High spin multiplicities in the ferromagnetic state are observed for these clusters indicating therein outstanding paramagnetic response.

  17. Analysis of proton and neutron pair breakings: High-spin structures of 124-127Te isotopes

    NASA Astrophysics Data System (ADS)

    Kumar, Vikas; Srivastava, P. C.; Ermamatov, M. J.; Morales, Irving O.

    2015-10-01

    In the present work recently available experimental data for high-spin states of four nuclei, Te12452, Te12552, Te12652, and Te12752, have been interpreted using state-of-the-art shell model calculations. The calculations have been performed in the 50-82 valence shell composed of 1g7/2, 2d5/2, 1h11/2, 3s1/2, and 2d3/2 orbitals. We have compared our results with the available experimental data for excitation energies and transition probabilities, including high-spin states. The results are in reasonable agreement with the available experimental data. The wave functions, particularly, the specific proton and neutron configurations which are involved to generate the angular momentum along the yrast lines are discussed. We have also estimated overall contribution of three-body forces in the energy level shifting. Finally, results with modified effective interaction are also reported.

  18. Pseudogaps and the spin-bag approach to high- T sub c superconductivity

    SciTech Connect

    Kampf, A.; Schrieffer, J.R. )

    1990-04-01

    It is shown that antiferromagnetic spin fluctuations in a two-dimensional metal, such as heavily doped cuprate superconductors, lead to a pseudogap in the electronic spectrum. The spectral function evolves from one peak in the Fermi-liquid regime to two peaks, one for particles and one for holes. The self-energy of spin bags and their pairing interaction are calculated. These results are consistent with the corresponding results in the weakly doped ordered antiferromagnet.

  19. High-fidelity readout and control of a nuclear spin qubit in silicon.

    PubMed

    Pla, Jarryd J; Tan, Kuan Y; Dehollain, Juan P; Lim, Wee H; Morton, John J L; Zwanenburg, Floris A; Jamieson, David N; Dzurak, Andrew S; Morello, Andrea

    2013-04-18

    Detection of nuclear spin precession is critical for a wide range of scientific techniques that have applications in diverse fields including analytical chemistry, materials science, medicine and biology. Fundamentally, it is possible because of the extreme isolation of nuclear spins from their environment. This isolation also makes single nuclear spins desirable for quantum-information processing, as shown by pioneering studies on nitrogen-vacancy centres in diamond. The nuclear spin of a (31)P donor in silicon is very promising as a quantum bit: bulk measurements indicate that it has excellent coherence times and silicon is the dominant material in the microelectronics industry. Here we demonstrate electrical detection and coherent manipulation of a single (31)P nuclear spin qubit with sufficiently high fidelities for fault-tolerant quantum computing. By integrating single-shot readout of the electron spin with on-chip electron spin resonance, we demonstrate quantum non-demolition and electrical single-shot readout of the nuclear spin with a readout fidelity higher than 99.8 percent-the highest so far reported for any solid-state qubit. The single nuclear spin is then operated as a qubit by applying coherent radio-frequency pulses. For an ionized (31)P donor, we find a nuclear spin coherence time of 60 milliseconds and a one-qubit gate control fidelity exceeding 98 percent. These results demonstrate that the dominant technology of modern electronics can be adapted to host a complete electrical measurement and control platform for nuclear-spin-based quantum-information processing. PMID:23598342

  20. Stimulated quasiparticles in spin-split superconductors

    NASA Astrophysics Data System (ADS)

    Virtanen, P.; Heikkilä, T. T.; Bergeret, F. S.

    2016-01-01

    In superconductors spin split by an exchange field, thermal effects are coupled to spin transport. We show how an oscillating electromagnetic field in such systems creates spin imbalance, that can be detected with a spin-polarized probe. The sign and magnitude of the probe signal result from a competition between processes converting field-induced spin energy imbalance to spin imbalance, dominant at low frequencies, and microwave-driven pair breaking at high frequencies. In the presence of spin-flip scattering, we show that ac excitation also leads to multistabilities in the superconducting state.

  1. Low-energy electrodynamics of novel spin excitations in the quantum spin ice Yb₂Ti₂O₇.

    PubMed

    Pan, LiDong; Kim, Se Kwon; Ghosh, A; Morris, Christopher M; Ross, Kate A; Kermarrec, Edwin; Gaulin, Bruce D; Koohpayeh, S M; Tchernyshyov, Oleg; Armitage, N P

    2014-01-01

    In condensed matter systems, formation of long-range order (LRO) is often accompanied by new excitations. However, in many geometrically frustrated magnetic systems, conventional LRO is suppressed, while non-trivial spin correlations are still observed. A natural question to ask is then what is the nature of the excitations in this highly correlated state without broken symmetry? Frequently, applying a symmetry breaking field stabilizes excitations whose properties reflect certain aspects of the anomalous state without LRO. Here we report a THz spectroscopy study of novel excitations in quantum spin ice Yb2Ti2O7 under a <001> directed magnetic field. At large positive fields, both right- and left-handed magnon and two-magnon-like excitations are observed. The g-factors of these excitations are dramatically enhanced in the low-field limit, showing a crossover of these states into features consistent with the quantum string-like excitations proposed to exist in quantum spin ice in small <001> fields. PMID:25233136

  2. Repulsively bound exciton-biexciton states in high-spin fermions in optical lattices

    SciTech Connect

    Argueelles, A.; Santos, L.

    2011-03-15

    We show that the interplay between spin-changing collisions and quadratic Zeeman coupling provides a mechanism for the formation of repulsively bound composites in high-spin fermions, which we illustrate by considering spin flips in an initially polarized hard-core one-dimensional Mott insulator of spin-3/2 fermions. We show that after the flips the dynamics is characterized by the creation of two types of exciton-biexciton composites. We analyze the conditions for the existence of these bound states and discuss their intriguing properties. In particular we show that the effective mass and stability of the composites depends nontrivially on spin-changing collisions, on the quadratic Zeeman effect, and on the initial exciton localization. Finally, we show that the composites may remain stable against inelastic collisions, opening the possibility of interesting quantum composite phases.

  3. High-resolution NMR spectroscopy of biological tissues usingprojected Magic Angle Spinning

    SciTech Connect

    Martin, Rachel W.; Jachmann, Rebecca C.; Sakellariou, Dimitris; Nielsen, Ulla Gro; Pines, Alexander

    2005-01-27

    High-resolution NMR spectra of materials subject toanisotropic broadening are usually obtained by rotating the sample aboutthe magic angle, which is 54.7 degrees to the static magnetic field. Inprojected Magic Angle Spinning (p-MAS), the sample is spun about twoangles, neither of which is the magic angle. This provides a method ofobtaining isotropic spectra while spinning at shallow angles. The p-MASexperiment may be used in situations where spinning the sample at themagic angle is not possible due to geometric or other constraints,allowing the choice of spinning angle to be determined by factors such asthe shape of the sample, rather than by the spin physics. The applicationof this technique to bovine tissue samples is demonstrated as a proof ofprinciple for future biological or medical applications.

  4. A high-performance Fortran code to calculate spin- and parity-dependent nuclear level densities

    NASA Astrophysics Data System (ADS)

    Sen'kov, R. A.; Horoi, M.; Zelevinsky, V. G.

    2013-01-01

    A high-performance Fortran code is developed to calculate the spin- and parity-dependent shell model nuclear level densities. The algorithm is based on the extension of methods of statistical spectroscopy and implies exact calculation of the first and second Hamiltonian moments for different configurations at fixed spin and parity. The proton-neutron formalism is used. We have applied the method for calculating the level densities for a set of nuclei in the sd-, pf-, and pf+g- model spaces. Examples of the calculations for 28Si (in the sd-model space) and 64Ge (in the pf+g-model space) are presented. To illustrate the power of the method we estimate the ground state energy of 64Ge in the larger model space pf+g, which is not accessible to direct shell model diagonalization due to the prohibitively large dimension, by comparing with the nuclear level densities at low excitation energy calculated in the smaller model space pf. Program summaryProgram title: MM Catalogue identifier: AENM_v1_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AENM_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: Standard CPC licence, http://cpc.cs.qub.ac.uk/licence/licence.html No. of lines in distributed program, including test data, etc.: 193181 No. of bytes in distributed program, including test data, etc.: 1298585 Distribution format: tar.gz Programming language: Fortran 90, MPI. Computer: Any architecture with a Fortran 90 compiler and MPI. Operating system: Linux. RAM: Proportional to the system size, in our examples, up to 75Mb Classification: 17.15. External routines: MPICH2 (http://www.mcs.anl.gov/research/projects/mpich2/) Nature of problem: Calculating of the spin- and parity-dependent nuclear level density. Solution method: The algorithm implies exact calculation of the first and second Hamiltonian moments for different configurations at fixed spin and parity. The code is parallelized using the Message

  5. High-Speed Magic-Angle Spinning 13C MAS NMR Spectra of Adamantane: Self-Decoupling of the Heteronuclear Scalar Interaction and Proton Spin Diffusion

    NASA Astrophysics Data System (ADS)

    Ernst, Matthias; Verhoeven, Aswin; Meier, Beat H.

    1998-02-01

    We have investigated the carbon line shape of solid adamantane under high-speed magic-angle sample spinning (MAS) acquired without proton decoupling. The CH-group shows a spinning-speed-dependent line broadening while the CH2-group consists of a spinning-speed-independent sharp component and a spinning-speed-dependent broader part. These phenomena can be explained by self-decoupling of theJ-interaction due to proton spin diffusion. Such a self-decoupling process can be described by a magnetization exchange process between the multiplet lines. Changing the spin-diffusion rate constant by off-resonance irradiation of the protons allows us to observe the full range from slow exchange to coalescence to fast exchange of the carbon spectra. One of the multiplet components in the CH2-group corresponds to a group spin of the protons of zero and therefore does not couple to the other protons. This gives rise to the sharp central line. The magnetization exchange rate constant between the different multiplet lines can be determined from the spectra and is a measure for the spinning-speed-dependent proton spin-diffusion rate constant. Even at an MAS speed of 30 kHz, proton spin diffusion is still observable despite the relatively weak intermolecular proton dipolar-coupling network in adamantane which results in a static proton line width of only 14 kHz (full width at half height).

  6. Formation of quantum spin Hall state on Si surface and energy gap scaling with strength of spin orbit coupling

    SciTech Connect

    Zhou, Miao; Ming, Wenmei; Liu, Zheng; Wang, Zhengfei; Yao, Yugui; Liu, Feng

    2014-11-19

    For potential applications in spintronics and quantum computing, it is desirable to place a quantum spin Hall insulator [i.e., a 2D topological insulator (TI)] on a substrate while maintaining a large energy gap. Here, we demonstrate a unique approach to create the large-gap 2D TI state on a semiconductor surface, based on first-principles calculations and effective Hamiltonian analysis. We show that when heavy elements with strong spin orbit coupling (SOC) such as Bi and Pb atoms are deposited on a patterned H-Si(111) surface into a hexagonal lattice, they exhibit a 2D TI state with a large energy gap of ≥0.5 eV. The TI state arises from an intriguing substrate orbital filtering effect that selects a suitable orbital composition around the Fermi level, so that the system can be matched onto a four-band effective model Hamiltonian. Furthermore, it is found that within this model, the SOC gap does not increase monotonically with the increasing strength of SOC. These interesting results may shed new light in future design and fabrication of large-gap topological quantum states.

  7. Formation of quantum spin Hall state on Si surface and energy gap scaling with strength of spin orbit coupling

    DOE PAGESBeta

    Zhou, Miao; Ming, Wenmei; Liu, Zheng; Wang, Zhengfei; Yao, Yugui; Liu, Feng

    2014-11-19

    For potential applications in spintronics and quantum computing, it is desirable to place a quantum spin Hall insulator [i.e., a 2D topological insulator (TI)] on a substrate while maintaining a large energy gap. Here, we demonstrate a unique approach to create the large-gap 2D TI state on a semiconductor surface, based on first-principles calculations and effective Hamiltonian analysis. We show that when heavy elements with strong spin orbit coupling (SOC) such as Bi and Pb atoms are deposited on a patterned H-Si(111) surface into a hexagonal lattice, they exhibit a 2D TI state with a large energy gap of ≥0.5more » eV. The TI state arises from an intriguing substrate orbital filtering effect that selects a suitable orbital composition around the Fermi level, so that the system can be matched onto a four-band effective model Hamiltonian. Furthermore, it is found that within this model, the SOC gap does not increase monotonically with the increasing strength of SOC. These interesting results may shed new light in future design and fabrication of large-gap topological quantum states.« less

  8. Formation of quantum spin Hall state on Si surface and energy gap scaling with strength of spin orbit coupling

    PubMed Central

    Zhou, Miao; Ming, Wenmei; Liu, Zheng; Wang, Zhengfei; Yao, Yugui; Liu, Feng

    2014-01-01

    For potential applications in spintronics and quantum computing, it is desirable to place a quantum spin Hall insulator [i.e., a 2D topological insulator (TI)] on a substrate while maintaining a large energy gap. Here, we demonstrate a unique approach to create the large-gap 2D TI state on a semiconductor surface, based on first-principles calculations and effective Hamiltonian analysis. We show that when heavy elements with strong spin orbit coupling (SOC) such as Bi and Pb atoms are deposited on a patterned H-Si(111) surface into a hexagonal lattice, they exhibit a 2D TI state with a large energy gap of ≥0.5 eV. The TI state arises from an intriguing substrate orbital filtering effect that selects a suitable orbital composition around the Fermi level, so that the system can be matched onto a four-band effective model Hamiltonian. Furthermore, it is found that within this model, the SOC gap does not increase monotonically with the increasing strength of SOC. These interesting results may shed new light in future design and fabrication of large-gap topological quantum states. PMID:25407432

  9. High energy physics

    SciTech Connect

    Kernan, A.; Shen, B.C.; Ma, E.

    1997-07-01

    This proposal is for the continuation of the High Energy Physics program at the University of California at Riverside. In hadron collider physics the authors will complete their transition from experiment UA1 at CERN to the DZERO experiment at Fermilab. On experiment UA1 their effort will concentrate on data analysis at Riverside. At Fermilab they will coordinate the high voltage system for all detector elements. They will also carry out hardware/software development for the D0 muon detector. The TPC/Two-Gamma experiment has completed its present phase of data-taking after accumulating 160 pb{sup {minus}}1 of luminosity. The UC Riverside group will continue data and physics analysis and make minor hardware improvement for the high luminosity run. The UC Riverside group is participating in design and implementation of the data acquisition system for the OPAL experiment at LEP. Mechanical and electronics construction of the OPAL hadron calorimeter strip readout system is proceeding on schedule. Data analysis and Monte Carlo detector simulation efforts are proceeding in preparation for the first physics run when IEP operation comenses in fall 1989.

  10. Puncture Initial Data for Highly Spinning Black-Hole Binaries

    NASA Astrophysics Data System (ADS)

    Ruchlin, Ian; Healy, James; Lousto, Carlos; Zlochower, Yosef

    2015-04-01

    Accretion arguments suggest that some astrophysical black-holes will possess nearly extremal spins. It is expected that gravitational wave signals from orbiting and merging black-hole binaries will be detected by Advanced LIGO in the next few years. Accurate waveform models are needed to interpret detector data. We solve the Hamiltonian and momentum constraints of General Relativity representing two black-holes with nearly extremal spins and ultra-relativistic boosts in the puncture formalism using spectral methods in the Cactus/Einstein Toolkit framework. We use a non-conformally-flat ansatz with an attenuated superposition of two conformally rescaled Lorentz-boosted-Kerr 3-metrics and their corresponding conformal extrinsic curvatures. The initial data are evolved in time using moving punctures in the BSSN and Z4 formalisms. We compare with the standard Bowen-York conformally-flat ansatz, finding an order of magnitude smaller burst of spurious radiation.

  11. High Energy Astrophysics Mission

    NASA Technical Reports Server (NTRS)

    White, Nicholas E.; Ormes, Jonathan F. (Technical Monitor)

    2000-01-01

    The nature of gravity and its relationship to the other three forces and to quantum theory is one of the major challenges facing us as we begin the new century. In order to make progress we must challenge the current theories by observing the effects of gravity under the most extreme conditions possible. Black holes represent one extreme, where the laws of physics as we understand them break down. The Universe as whole is another extreme, where its evolution and fate is dominated by the gravitational influence of dark matter and the nature of the Cosmological constant. The early universe represents a third extreme, where it is thought that gravity may somehow be unified with the other forces. NASA's "Cosmic Journeys" program is part of a NASA/NSF/DoE tri-agency initiative designed to observe the extremes of gravity throughout the universe. This program will probe the nature of black holes, ultimately obtaining a direct image of the event horizon. It will investigate the large scale structure of the Universe to constrain the location and nature of dark matter and the nature of the cosmological constant. Finally it will search for and study the highest energy processes, that approach those found in the early universe. I will outline the High Energy Astrophysics part of this program.

  12. High fidelity readout of a single electron spin

    NASA Astrophysics Data System (ADS)

    Keselman, Anna; Glickman, Yinnon; Akerman, Nitzan; Kotler, Shlomi; Dallal, Yehonatan; Ozeri, Roee

    2010-03-01

    We use the two spin states of the valence electron of a single trapped ^88Sr^+ ion as a physical qubit implementation. For qubit readout one of the qubit states is shelved to a metastable D level using a narrow linewidth 674nm diode laser followed by state-selective fluorescence detection. Careful analysis of the resulting photon detection statistics allows for a minimal detection error of 2 . 10-3, compatible with recent estimates of the fault-tolerance required error threshold.

  13. High-spin configuration of Mn in Bi2Se3 three-dimensional topological insulator

    NASA Astrophysics Data System (ADS)

    Wolos, Agnieszka; Drabinska, Aneta; Borysiuk, Jolanta; Sobczak, Kamil; Kaminska, Maria; Hruban, Andrzej; Strzelecka, Stanislawa G.; Materna, Andrzej; Piersa, Miroslaw; Romaniec, Magdalena; Diduszko, Ryszard

    2016-12-01

    Electron paramagnetic resonance was used to investigate Mn impurity in Bi2Se3 topological insulator grown by the vertical Bridgman method. Mn in high-spin S=5/2, Mn2+, configuration was detected regardless of the conductivity type of the host material. This means that Mn2+(d5) energy level is located within the valence band, and Mn1+(d6) energy level is outside the energy gap of Bi2Se3. The electron paramagnetic resonance spectrum of Mn2+ in Bi2Se3 is characterized by the isotropic g-factor |g|=1.91 and large axial parameter D=-4.20 GHz h. This corresponds to the zero-field splitting of the Kramers doublets equal to 8.4 GHz h and 16.8 GHz h, respectively, which is comparable to the Zeeman splitting for the X-band. Mn in Bi2Se3 acts as an acceptor, effectively reducing native-high electron concentration, compensating selenium vacancies, and resulting in p-type conductivity. However, Mn-doping simultaneously favors formation of native donor defects, most probably selenium vacancies. For high Mn-doping it may lead to the resultant n-type conductivity related with strong non-stoichiometry and degradation of the crystal structure - switching from Bi2Se3 to BiSe phase.

  14. High density spin noise spectroscopy with squeezed light

    NASA Astrophysics Data System (ADS)

    Lucivero, Vito Giovanni; Jiménez-Martínez, Ricardo; Kong, Jia; Mitchell, Morgan

    2016-05-01

    Spin noise spectroscopy (SNS) has recently emerged as a powerful technique for determining physical properties of an unperturbed spin system from its power noise spectrum both in atomic and solid state physics. In the presence of a transverse magnetic field, we detect spontaneous spin fluctuations of a dense Rb vapor via Faraday rotation of an off-resonance probe beam, resulting in the excess of spectral noise at the Larmor frequency over a white photon shot-noise background. We report quantum enhancement of the signal-to-noise ratio via polarization squeezing of the probe beam up to 3dB over the full density range up to n = 1013 atoms cm-3, covering practical conditions used in optimized SNS experiments. Furthermore, we show that squeezing improves the trade-off between statistical sensitivity and systematic errors due to line broadening, a previously unobserved quantum advantage. Finally, we present a novel theoretical model on quantum limits of noise spectroscopies by defining a standard quantum limit under optimized regimes and by discussing the conditions of its overcoming due to squeezing.

  15. Collective spin 1 singlet phase in high-pressure oxygen

    PubMed Central

    Crespo, Yanier; Fabrizio, Michele; Scandolo, Sandro; Tosatti, Erio

    2014-01-01

    Oxygen, one of the most common and important elements in nature, has an exceedingly well-explored phase diagram under pressure, up to and beyond 100 GPa. At low temperatures, the low-pressure antiferromagnetic phases below 8 GPa where O2 molecules have spin S = 1 are followed by the broad apparently nonmagnetic ε phase from about 8 to 96 GPa. In this phase, which is our focus, molecules group structurally together to form quartets while switching, as believed by most, to spin S = 0. Here we present theoretical results strongly connecting with existing vibrational and optical evidence, showing that this is true only above 20 GPa, whereas the S = 1 molecular state survives up to about 20 GPa. The ε phase thus breaks up into two: a spinless ε0 (20−96 GPa), and another ε1 (8−20 GPa) where the molecules have S = 1 but possess only short-range antiferromagnetic correlations. A local spin liquid-like singlet ground state akin to some earlier proposals, and whose optical signature we identify in existing data, is proposed for this phase. Our proposed phase diagram thus has a first-order phase transition just above 20 GPa, extending at finite temperature and most likely terminating into a crossover with a critical point near 30 GPa and 200 K. PMID:25002513

  16. Collective spin 1 singlet phase in high-pressure oxygen.

    PubMed

    Crespo, Yanier; Fabrizio, Michele; Scandolo, Sandro; Tosatti, Erio

    2014-07-22

    Oxygen, one of the most common and important elements in nature, has an exceedingly well-explored phase diagram under pressure, up to and beyond 100 GPa. At low temperatures, the low-pressure antiferromagnetic phases below 8 GPa where O2 molecules have spin S = 1 are followed by the broad apparently nonmagnetic ε phase from about 8 to 96 GPa. In this phase, which is our focus, molecules group structurally together to form quartets while switching, as believed by most, to spin S = 0. Here we present theoretical results strongly connecting with existing vibrational and optical evidence, showing that this is true only above 20 GPa, whereas the S = 1 molecular state survives up to about 20 GPa. The ε phase thus breaks up into two: a spinless ε0 (20-96 GPa), and another ε1 (8-20 GPa) where the molecules have S = 1 but possess only short-range antiferromagnetic correlations. A local spin liquid-like singlet ground state akin to some earlier proposals, and whose optical signature we identify in existing data, is proposed for this phase. Our proposed phase diagram thus has a first-order phase transition just above 20 GPa, extending at finite temperature and most likely terminating into a crossover with a critical point near 30 GPa and 200 K. PMID:25002513

  17. Numerical relativity and high energy physics: Recent developments

    NASA Astrophysics Data System (ADS)

    Berti, Emanuele; Cardoso, Vitor; Crispino, Luis C. B.; Gualtieri, Leonardo; Herdeiro, Carlos; Sperhake, Ulrich

    2016-07-01

    We review recent progress in the application of numerical relativity techniques to astrophysics and high-energy physics. We focus on recent developments regarding the spin evolution in black hole binaries, high-energy black hole collisions, compact object solutions in scalar-tensor gravity, superradiant instabilities, hairy black hole solutions in Einstein’s gravity coupled to fundamental fields, and the possibility to gain insight into these phenomena using analog gravity models.

  18. High-resolution electron microscopy in spin pumping NiFe/Pt interfaces

    SciTech Connect

    Ley Domínguez, D. Sáenz-Hernández, R. J.; Faudoa Arzate, A.; Arteaga Duran, A. I.; Ornelas Gutiérrez, C. E.; Solís Canto, O.; Botello-Zubiate, M. E.; Rivera-Gómez, F. J.; Matutes-Aquino, J. A.; Azevedo, A.; Silva, G. L. da; Rezende, S. M.

    2015-05-07

    In order to understand the effect of the interface on the spin pumping and magnetic proximity effects, high resolution transmission electron microscopy and ferromagnetic resonance (FMR) were used to analyze Py/Pt bilayer and Pt/Py/Pt trilayer systems. The samples were deposited by dc magnetron sputtering at room temperature on Si (001) substrates. The Py layer thickness was fixed at 12 nm in all the samples and the Pt thickness was varied in a range of 0–23 nm. A diffusion zone of approximately 8 nm was found in the Py/Pt interfaces and confirmed by energy dispersive X-ray microanalysis. The FMR measurements show an increase in the linewidth and a shift in the ferromagnetic resonance field, which reach saturation.

  19. High-resolution electron microscopy in spin pumping NiFe/Pt interfaces

    NASA Astrophysics Data System (ADS)

    Ley Domínguez, D.; Sáenz-Hernández, R. J.; Faudoa Arzate, A.; Arteaga Duran, A. I.; Ornelas Gutiérrez, C. E.; Solís Canto, O.; Botello-Zubiate, M. E.; Rivera-Gómez, F. J.; Azevedo, A.; da Silva, G. L.; Rezende, S. M.; Matutes-Aquino, J. A.

    2015-05-01

    In order to understand the effect of the interface on the spin pumping and magnetic proximity effects, high resolution transmission electron microscopy and ferromagnetic resonance (FMR) were used to analyze Py/Pt bilayer and Pt/Py/Pt trilayer systems. The samples were deposited by dc magnetron sputtering at room temperature on Si (001) substrates. The Py layer thickness was fixed at 12 nm in all the samples and the Pt thickness was varied in a range of 0-23 nm. A diffusion zone of approximately 8 nm was found in the Py/Pt interfaces and confirmed by energy dispersive X-ray microanalysis. The FMR measurements show an increase in the linewidth and a shift in the ferromagnetic resonance field, which reach saturation.

  20. Two successive spin transitions in a wide range of pressure and coexistence of high- and low-spin states in clinoferrosilite FeSiO3

    NASA Astrophysics Data System (ADS)

    Dyachenko, Alexey A.; Shorikov, Alexey O.; Lukoyanov, Alexey V.; Anisimov, Vladimir I.

    2016-06-01

    We present a theoretical study of spectral and magnetic properties of clinoferrosilite FeSiO3. Within the DFT+DMFT method combining local density approximation with dynamical mean-field theory FeSiO3 was investigated in a wide range of pressure and temperature including the lower Earth's mantle conditions. For clinoferrosilite, which crystallizes in a monoclinic crystal structure, we predict two high-spin to low-spin transitions under pressure in the Fe-3 d shell with a crossover region at moderate temperatures, which becomes much broader at higher temperatures. An analysis of the Fe electronic configurations reveals that in clinoferrosilite the low- and high-spin states are predominantly involved and coexist in the spin crossover region, while a small amount of the intermediate spin states appears only at very high pressures and can be attributed to the distorted crystal structure of clinoferrosilite FeSiO3.

  1. Spin-wave-driven high-speed domain-wall motions in soft magnetic nanotubes

    SciTech Connect

    Yang, Jaehak; Yoo, Myoung-Woo; Kim, Sang-Koog

    2015-10-28

    We report on a micromagnetic simulation study of interactions between propagating spin waves and a head-to-head domain wall in geometrically confined magnetic nanotubes. We found that incident spin waves of specific frequencies can lead to sufficiently high-speed (on the order of a few hundreds of m/s or higher) domain-wall motions in the same direction as that of the incident spin-waves. The domain-wall motions and their speed vary remarkably with the frequency and the amplitude of the incident spin-waves. High-speed domain-wall motions originate from the transfer torque of spin waves' linear momentum to the domain wall, through the partial or complete reflection of the incident spin waves from the domain wall. This work provides a fundamental understanding of the interaction of the spin waves with a domain wall in the magnetic nanotubes as well as a route to all-magnetic control of domain-wall motions in the magnetic nanoelements.

  2. High energy scattering of Dirac particles on smooth potentials

    NASA Astrophysics Data System (ADS)

    Han, Nguyen Suan; Dung, Le Anh; Xuan, Nguyen Nhu; Thang, Vu Toan

    2016-08-01

    The derivation of the Glauber type representation for the high energy scattering amplitude of particles of spin 1/2 is given within the framework of the Dirac equation in the Foldy-Wouthuysen (FW) representation and two-component formalism. The differential cross-sections on the Yukawa and Gaussian potentials are also considered and discussed.

  3. Inevitable inflation in Einstein-Cartan theory with improved energy-momentum tensor with spin

    NASA Technical Reports Server (NTRS)

    Fennelly, A. J.; Bradas, James C.; Smalley, Larry L.

    1988-01-01

    Generalized, or power-law, inflation is shown to necessarily exist for a simple, anisotropic, (Bianchi Type-1) cosmology in the Einstein-Cartan gravitational theory with the Ray-Smalley improved energy momentum tensor with spin. Formal solution of the EC field equations with the fluid equations of motion explicitly shows inflation caused by the RS spin angular kinetic energy density. Shear is not effective in preventing inflation in the ECRS model. The relation between fluid vorticity, torsion, reference axis rotation, and shear ellipsoid precession shows through clearly.

  4. Spin in Hadron Reactions

    SciTech Connect

    Aidala, Christine A.

    2009-08-04

    The Relativistic Heavy Ion Collider (RHIC) has brought the study of spin effects in hadronic collisions to a new energy regime. In conjunction with other experiments at facilities around the world, much can be learned from the high-energy polarized proton collisions RHIC provides, allowing the collider to serve as a powerful tool to continue to understand the rich subtleties and surprises of spin effects in QCD, some of which were originally discovered more than three decades ago.

  5. Coherently coupling distinct spin ensembles through a high-Tc superconducting resonator

    NASA Astrophysics Data System (ADS)

    Ghirri, A.; Bonizzoni, C.; Troiani, F.; Buccheri, N.; Beverina, L.; Cassinese, A.; Affronte, M.

    2016-06-01

    The problem of coupling multiple spin ensembles through cavity photons is revisited by using (3,5-dichloro-4-pyridyl)bis(2,4,6-trichlorophenyl)methyl (PyBTM) organic radicals and a high-Tc superconducting coplanar resonator. An exceptionally strong coupling is obtained and up to three spin ensembles are simultaneously coupled. The ensembles are made physically distinguishable by chemically varying the g factor and by exploiting the inhomogeneities of the applied magnetic field. The coherent mixing of the spin and field modes is demonstrated by the observed multiple anticrossing, along with the simulations performed within the input-output formalism, and quantified by suitable entropic measures.

  6. High-accuracy gravitational waveforms for binary black hole mergers with nearly extremal spins

    NASA Astrophysics Data System (ADS)

    Lovelace, Geoffrey; Boyle, Michael; Scheel, Mark A.; Szilágyi, Béla

    2012-02-01

    Motivated by the possibility of observing gravitational waves from merging black holes whose spins are nearly extremal (i.e. 1 in dimensionless units), we present numerical waveforms from simulations of merging black holes with the highest spins simulated to date: (1) a 25.5-orbit inspiral, merger and ringdown of two holes with equal masses and spins of magnitude 0.97 aligned with the orbital angular momentum; and (2) a previously reported 12.5-orbit inspiral, merger and ringdown of two holes with equal masses and spins of magnitude 0.95 anti-aligned with the orbital angular momentum. First, we consider the horizon mass and spin evolution of the new aligned-spin simulation. During the inspiral, the horizon area and spin evolve in remarkably close agreement with Alvi's analytic predictions, and the remnant hole's final spin agrees reasonably well with several analytic predictions. We also find that the total energy emitted by a real astrophysical system with these parameters—almost all of which is radiated during the time included in this simulation—would be 10.952% of the initial mass at infinite separation. Second, we consider the gravitational waveforms for both simulations. After estimating their uncertainties, we compare the waveforms to several post-Newtonian approximants, finding significant disagreement well before merger, although the phase of the TaylorT4 approximant happens to agree remarkably well with the numerical prediction in the aligned-spin case. We find that the post-Newtonian waveforms have sufficient uncertainty that hybridized waveforms will require far longer numerical simulations (in the absence of improved post-Newtonian waveforms) for accurate parameter estimation of low-mass binary systems.

  7. Scaled Opposite Spin Second Order Moller-Plesset Correlation Energy: An Economical Electronic Structure Method

    SciTech Connect

    Jung, Yousung; Lochan, Rohini C.; Dutoi, Anthony D.; Head-Gordon, Martin

    2004-08-02

    A simplified approach to treating the electron correlation energy is suggested in which only the alpha-beta component of the second order Moller-Plesset energy is evaluated, and then scaled by an empirical factor which is suggested to be 1.3. This scaled opposite spin second order energy (SOS-MP2) yields results for relative energies and derivative properties that are statistically improved over the conventional MP2 method. Furthermore, the SOS-MP2 energy can be evaluated without the 5th order computational steps associated with MP2 theory, even without exploiting any spatial locality. A 4th order algorithm is given for evaluating the opposite spin MP2 energy using auxiliary basis expansions, and a Laplace approach, and timing comparisons are given.

  8. Nonuniqueness of magnetic fields and energy derivatives in spin-polarized density functional theory

    NASA Astrophysics Data System (ADS)

    Gál, T.; Ayers, P. W.; De Proft, F.; Geerlings, P.

    2009-10-01

    The effect of the recently uncovered nonuniqueness of the external magnetic field B(r⃑) corresponding to a given pair of density n(r⃑) and spin density ns(r⃑) on the derivative of the energy functional of spin-polarized density functional theory, and its implications for the definition of chemical reactivity descriptors, is examined. For ground states, the nonuniqueness of B(r⃑) implies the nondifferentiability of the energy functional Ev,B[n,ns] with respect to ns(r⃑). It is shown, on the other hand, that this nonuniqueness allows the existence of the one-sided derivatives of Ev,B[n,ns] with respect to ns(r⃑). Although the N-electron ground state can always be obtained from the minimization of Ev,B[n,ns] without any constraint on the spin number Ns=∫ns(r⃑)dr⃑, the Lagrange multiplier μs associated with the fixation of Ns does not vanish even for ground states. μs is identified as the left- or right-side derivative of the total energy with respect to Ns, which justifies the interpretation of μs as a (spin) chemical potential. This is relevant not only for the spin-polarized generalization of conceptual density functional theory, the spin chemical potential being one of the elementary reactivity descriptors, but also for the extension of the thermodynamical analogy of density functional theory for the spin-polarized case. For higher-order reactivity indices, B(r⃑)'s nonuniqueness has similar implications as for μs, leading to a split of the indices with respect to Ns into one-sided reactivity descriptors.

  9. FSU High Energy Physics

    SciTech Connect

    Prosper, Harrison B.; Adams, Todd; Askew, Andrew; Berg, Bernd; Blessing, Susan K.; Okui, Takemichi; Owens, Joseph F.; Reina, Laura; Wahl, Horst D.

    2014-12-01

    The High Energy Physics group at Florida State University (FSU), which was established in 1958, is engaged in the study of the fundamental constituents of matter and the laws by which they interact. The group comprises theoretical and experimental physicists, who sometimes collaborate on projects of mutual interest. The report highlights the main recent achievements of the group. Significant, recent, achievements of the group’s theoretical physicists include progress in making precise predictions in the theory of the Higgs boson and its associated processes, and in the theoretical understanding of mathematical quantities called parton distribution functions that are related to the structure of composite particles such as the proton. These functions are needed to compare data from particle collisions, such as the proton-proton collisions at the CERN Large Hadron Collider (LHC), with theoretical predictions. The report also describes the progress in providing analogous functions for heavy nuclei, which find application in neutrino physics. The report highlights progress in understanding quantum field theory on a lattice of points in space and time (an area of study called lattice field theory), the progress in constructing several theories of potential new physics that can be tested at the LHC, and interesting new ideas in the theory of the inflationary expansion of the very early universe. The focus of the experimental physicists is the Compact Muon Solenoid (CMS) experiment at CERN. The report, however, also includes results from the D0 experiment at Fermilab to which the group made numerous contributions over a period of many years. The experimental group is particularly interested in looking for new physics at the LHC that may provide the necessary insight to extend the standard model (SM) of particle physics. Indeed, the search for new physics is the primary task of contemporary particle physics, one motivated by the need to explain certain facts, such as the

  10. High Spin Polarization at Ferromagnetic Metal-Organic Interfaces: A Generic Property.

    PubMed

    Djeghloul, Fatima; Gruber, Manuel; Urbain, Etienne; Xenioti, Dimitra; Joly, Loic; Boukari, Samy; Arabski, Jacek; Bulou, Hervé; Scheurer, Fabrice; Bertran, François; Le Fèvre, Patrick; Taleb-Ibrahimi, Amina; Wulfhekel, Wulf; Garreau, Guillaume; Hajjar-Garreau, Samar; Wetzel, Patrick; Alouani, Mebarek; Beaurepaire, Eric; Bowen, Martin; Weber, Wolfgang

    2016-07-01

    A high spin polarization of states around the Fermi level, EF, at room temperature has been measured in the past at the interface between a few molecular candidates and the ferromagnetic metal Co. Is this promising property for spintronics limited to these candidates? Previous reports suggested that certain conditions, such as strong ferromagnetism, i.e., a fully occupied spin-up d band of the ferromagnet, or the presence of π bonds on the molecule, i.e., molecular conjugation, needed to be met. What rules govern the presence of this property? We have performed spin-resolved photoemission spectroscopy measurements on a variety of such interfaces. We find that this property is robust against changes to the molecule and ferromagnetic metal's electronic properties, including the aforementioned conditions. This affirms the generality of highly spin-polarized states at the interface between a ferromagnetic metal and a molecule and augurs bright prospects toward integrating these interfaces within organic spintronic devices. PMID:27266579

  11. Coherent manipulation of an ensemble of nuclear spins in diamond for high precision rotation sensing

    NASA Astrophysics Data System (ADS)

    Jaskula, Jean-Christophe; Saha, Kasturi; Ajoy, Ashok; Cappellaro, Paola

    2016-05-01

    Gyroscopes find wide applications in everyday life from navigation and inertial sensing to rotation sensors in hand-held devices and automobiles. Current devices, based on either atomic or solid-state systems, impose a choice between long-time stability and high sensitivity in a miniaturized system. We are building a solid-state spin gyroscope associated with the Nitrogen-Vacancy (NV) centers in diamond take advantage of the efficient optical initialization and measurement offered by the NV electronic spin and the stability and long coherence time of the nuclear spin, which is preserved even at high defect density. In addition, we also investigate electro-magnetic noise monitoring and feedback schemes based on the coupling between the NV electronic and nuclear spin to achieve higher stability.

  12. Ultrafast high-fidelity initialization of a quantum-dot spin qubit without magnetic fields

    NASA Astrophysics Data System (ADS)

    Mar, Jonathan D.; Baumberg, Jeremy J.; Xu, Xiulai; Irvine, Andrew C.; Williams, David A.

    2014-12-01

    We demonstrate the initialization of a single quantum-dot hole spin with high fidelity (lower bound >97 %), on picosecond time scales, and without the need for magnetic fields. Using the initialization scheme based on rapid electric-field ionization of a resonantly excited exciton, this is achieved by employing a self-assembled quantum dot with a low conduction-to-valence band offset ratio, allowing control of the relative electron and hole tunneling rates over three orders of magnitude. This large difference in tunneling rates could permit spin-storage efficiencies >99.5 % by fast-switching to a low electric-field condition. Our results may provide a practical route towards ultrafast high-fidelity initialization of individual quantum-dot hole spins for the implementation of quantum error correction in a scalable spin-based quantum computer.

  13. High energy plasma accelerators

    SciTech Connect

    Tajima, T.

    1985-05-01

    Colinear intense laser beams ..omega../sub 0/, kappa/sub 0/ and ..omega../sub 1/, kappa/sub 1/ shone on a plasma with frequency separation equal to the electron plasma frequency ..omega../sub pe/ are capable of creating a coherent large longitudinal electric field E/sub L/ = mc ..omega../sub pe//e of the order of 1GeV/cm for a plasma density of 10/sup 18/ cm/sup -3/ through the laser beat excitation of plasma oscillations. Accompanying favorable and deleterious physical effects using this process for a high energy beat-wave accelerator are discussed: the longitudinal dephasing, pump depletion, the transverse laser diffraction, plasma turbulence effects, self-steepening, self-focusing, etc. The basic equation, the driven nonlinear Schroedinger equation, is derived to describe this system. Advanced accelerator concepts to overcome some of these problems are proposed, including the plasma fiber accelerator of various variations. An advanced laser architecture suitable for the beat-wave accelerator is suggested. Accelerator physics issues such as the luminosity are discussed. Applications of the present process to the current drive in a plasma and to the excitation of collective oscillations within nuclei are also discussed.

  14. High energy physics

    SciTech Connect

    Kernan, A.; Shen, B.C.; Ma, E.

    1997-07-01

    This proposal is for the continuation of the High Energy Physics Program at the University of California, Riverside. In 1990, we will concentrate on analysis of LEP data from the OPAL detector. We expect to record 10{sup 5} Z`s by the end of 1989 and 10{sup 6} in 1990. This data will be used to measure the number of quark-lepton families in the universe. In the second half of 1990 we will also be occupied with the installation of the D-Zero detector in the Tevatron Collider and the preparation of software for the 1991 run. A new initiative made possible by generous university support is a laboratory for detector development at UCR. The focus will be on silicon strip tracking detectors both for the D-Zero upgrade and for SSC physics. The theory program will pursue further various mass-generating radiative mechanisms for understanding small quark and lepton masses as well as some novel phenomenological aspects of supersymmetry.

  15. Spin-injection spectroscopy of a spin-orbit coupled Fermi gas.

    PubMed

    Cheuk, Lawrence W; Sommer, Ariel T; Hadzibabic, Zoran; Yefsah, Tarik; Bakr, Waseem S; Zwierlein, Martin W

    2012-08-31

    The coupling of the spin of electrons to their motional state lies at the heart of recently discovered topological phases of matter. Here we create and detect spin-orbit coupling in an atomic Fermi gas, a highly controllable form of quantum degenerate matter. We directly reveal the spin-orbit gap via spin-injection spectroscopy, which characterizes the energy-momentum dispersion and spin composition of the quantum states. For energies within the spin-orbit gap, the system acts as a spin diode. We also create a spin-orbit coupled lattice and probe its spinful band structure, which features additional spin gaps and a fully gapped spectrum. In the presence of s-wave interactions, such systems should display induced p-wave pairing, topological superfluidity, and Majorana edge states. PMID:23002844

  16. High-fidelity projective read-out of a solid-state spin quantum register.

    PubMed

    Robledo, Lucio; Childress, Lilian; Bernien, Hannes; Hensen, Bas; Alkemade, Paul F A; Hanson, Ronald

    2011-09-29

    Initialization and read-out of coupled quantum systems are essential ingredients for the implementation of quantum algorithms. Single-shot read-out of the state of a multi-quantum-bit (multi-qubit) register would allow direct investigation of quantum correlations (entanglement), and would give access to further key resources such as quantum error correction and deterministic quantum teleportation. Although spins in solids are attractive candidates for scalable quantum information processing, their single-shot detection has been achieved only for isolated qubits. Here we demonstrate the preparation and measurement of a multi-spin quantum register in a low-temperature solid-state system by implementing resonant optical excitation techniques originally developed in atomic physics. We achieve high-fidelity read-out of the electronic spin associated with a single nitrogen-vacancy centre in diamond, and use this read-out to project up to three nearby nuclear spin qubits onto a well-defined state. Conversely, we can distinguish the state of the nuclear spins in a single shot by mapping it onto, and subsequently measuring, the electronic spin. Finally, we show compatibility with qubit control: we demonstrate initialization, coherent manipulation and single-shot read-out in a single experiment on a two-qubit register, using techniques suitable for extension to larger registers. These results pave the way for a test of Bell's inequalities on solid-state spins and the implementation of measurement-based quantum information protocols. PMID:21937989

  17. Study of Low Energy Electron Inelastic Scattering Mechanisms Using Spin Sensitive Techniques

    NASA Astrophysics Data System (ADS)

    Hsu, Hongbing

    1995-01-01

    Spin sensitive electron spectroscopies were used to study low energy electron inelastic scattering from metal surfaces and thin films. In these experiments, a beam of spin polarized electrons from a GaAs source is directed on the sample surface, and the spin polarization and intensity are measured as a function of energy loss and scattering angle by a Mott electron polarimeter coupled with a concentric hemispherical energy analyzer. Systematic studies of the angular dependence of inelastically scattered electrons were conducted on a Cu(100) surface, and Mo/Cu(100), non-magnetized Fe/Cu(100), and Co/Cu(100) films. The polarization and intensity of scattered electrons were measured as function of energy loss and scattering angle. Further studies were also conducted on Ag(100) surface and amorphous Cu/Ag(100) films. From the experimental results, the angular distributions of dipole and impact scattered electrons can be determined individually and both are found to peak in the specular scattering direction. Preliminary studies were conducted on magnetized Co/Cu(100) films. The spin dependent scattering intensity asymmetry was measured, with a clearly observable peak at energy loss of ~1 eV, which coincides with the band splitting. The polarizations of secondary electrons produced by an unpolarized primary beam were also measured. The polarizations can be related to the band polarization of magnetized cobalt films.

  18. Scattering framework for two particles with isotropic spin-orbit coupling applicable to all energies

    NASA Astrophysics Data System (ADS)

    Guan, Q.; Blume, D.

    2016-08-01

    Previous work developed a K -matrix formalism applicable to positive energies for the scattering between two s -wave interacting particles with two internal states, isotropic spin-orbit coupling and vanishing center-of-mass momentum [H. Duan, L. You, and B. Gao, Phys. Rev. A 87, 052708 (2013)., 10.1103/PhysRevA.87.052708]. This work extends the formalism to the entire energy regime. Explicit solutions are obtained for the total angular momentum J =0 and 1 channels. The behavior of the partial cross sections in the negative energy regime is analyzed in detail. We find that the leading contributions to the partial cross sections at the negative energy thresholds are governed by the spin-orbit coupling strength kso and the mass ratio. The fact that these contributions are independent of the two-body scattering length as is a direct consequence of the effective reduction of the dimensionality, and hence of the density of states, near the scattering thresholds due to the single-particle spin-orbit coupling terms. The results are analytically continued to the energy regime where bound states exist. It is shown that our results are consistent with results obtained by alternative approaches. Our formulation, which can be regarded as an extension of the standard textbook partial wave decomposition, can be generalized to two-body systems with other types of spin-orbit coupling, including cases where the center-of-mass momentum does not vanish.

  19. Quantum corrections to energy of short spinning string in AdS{sub 5}

    SciTech Connect

    Tirziu, A.; Tseytlin, A. A.

    2008-09-15

    Motivated by a desire to shed light on the strong-coupling behavior of dimensions of short gauge-theory operators, we consider the famous example of folded spinning string in AdS{sub 5} in the limit of small semiclassical spin parameter S=(S/{radical}({lambda})). In this limit the string becomes short and is moving in a near-flat central region of AdS{sub 5}. Its energy scales with spin as E={radical}(2S)[a{sub 0}+a{sub 1}S+a{sub 2}S{sup 2}+...]. We explicitly compute the leading 1-loop quantum AdS{sub 5}xS{sup 5} superstring correction to the short string energy and show that the coefficient a{sub 0} is not renormalized from its classical value while a{sub 1} receives a nontrivial contribution containing {zeta}(3)

  20. The role of spin in cosmological models

    NASA Astrophysics Data System (ADS)

    Bedran, M. L.; Vasconcellos-Vaidya, E. P.

    1984-09-01

    The classical description of spin in a perfect fluid of Ray and Smalley (1982) and its energy-momentum-tensor formulation are applied to cosmological models. The Raychaudhuri equation for the evolution of a continuous matter distribution in hydrodynamic motion is analyzed, and the role of spin and torsion in the Einstein-Cartan theory of gravitation (Hehl et al., 1976) is compared to that of spin in general relativity. It is found that spin-spin interaction is significant only at extremely high densities, and that spin-vorticity interactions are of potential importance at high vorticity, as in the early moments of cosmological models.

  1. Efficiency of quantum energy teleportation within spin-1/2 particle pairs

    NASA Astrophysics Data System (ADS)

    Frey, Michael R.

    2016-03-01

    A protocol for quantum energy teleportation (QET) is known for a so-called minimal spin-1/2 particle pair model. We extend this protocol to explicitly admit quantum weak measurements at its first stage. The extended protocol is applied beyond the minimal model to spin-1/2 particle pairs whose Hamiltonians are of a general class characterized by orthogonal pairs of entangled eigenstates. The energy transfer efficiency of the extended QET protocol is derived for this setting, and we show that weaker measurement yields greater efficiency. In the minimal particle pair model, for example, the efficiency can be doubled by this means. We also show that the QET protocol's transfer efficiency never exceeds 100 %, supporting the understanding that quantum energy teleportation is, indeed, an energy transfer protocol, rather than a protocol for remotely catalyzing local extraction of system energy already present.

  2. Spin-out puts new spin on wind-energy technology

    NASA Astrophysics Data System (ADS)

    Johnston, Hamish

    2010-05-01

    The future of wind energy could involve huge blades spanning half a kilometre that generate compressed air - which is then piped into giant, underwater balloons. That is the dream of Seamus Garvey, a mechanical engineer at the University of Nottingham in the UK, who envisages using the pressurized air to inflate the balloons, nestling about 500 m below the surface of the sea. Electricity could then be generated, when required, by releasing the air to drive a set of turbines.

  3. High Energy Density Capacitors

    SciTech Connect

    2010-07-01

    BEEST Project: Recapping is developing a capacitor that could rival the energy storage potential and price of today’s best EV batteries. When power is needed, the capacitor rapidly releases its stored energy, similar to lightning being discharged from a cloud. Capacitors are an ideal substitute for batteries if their energy storage capacity can be improved. Recapping is addressing storage capacity by experimenting with the material that separates the positive and negative electrodes of its capacitors. These separators could significantly improve the energy density of electrochemical devices.

  4. Ultra-high energy probes of classicalization

    SciTech Connect

    Dvali, Gia; Gomez, Cesar E-mail: cesar.gomez@uam.es

    2012-07-01

    Classicalizing theories are characterized by a rapid growth of the scattering cross section. This growth converts these sort of theories in interesting probes for ultra-high energy experiments even at relatively low luminosity, such as cosmic rays or Plasma Wakefield accelerators. The microscopic reason behind this growth is the production of N-particle states, classicalons, that represent self-sustained lumps of soft Bosons. For spin-2 theories this is the quantum portrait of what in the classical limit are known as black holes. We emphasize the importance of this quantum picture which liberates us from the artifacts of the classical geometric limit and allows to scan a much wider landscape of experimentally-interesting quantum theories. We identify a phenomenologically-viable class of spin-2 theories for which the growth of classicalon production cross section can be as efficient as to compete with QCD cross section already at 100TeV energy, signaling production of quantum black holes with graviton occupation number N ∼ 10{sup 4}.

  5. Devices and process for high-pressure magic angle spinning nuclear magnetic resonance

    DOEpatents

    Hoyt, David W; Sears, Jr., Jesse A; Turcu, Romulus V.F.; Rosso, Kevin M; Hu, Jian Zhi

    2014-04-08

    A high-pressure magic angle spinning (MAS) rotor is detailed that includes a high-pressure sample cell that maintains high pressures exceeding 150 bar. The sample cell design minimizes pressure losses due to penetration over an extended period of time.

  6. Neutron Spin Structure Studies and Low-Energy Tests of the Standard Model at JLab

    SciTech Connect

    Jager, Kees de

    2008-10-13

    The most recent results on the spin structure of the neutron from Hall A are presented and discussed. Then, an overview is given of various experiments planned with the 12 GeV upgrade at Jefferson Lab to provide sensitive tests of the Standard Model at relatively low energies.

  7. Coulomb energy averaged over the nl{sup N}-atomic states with a definite spin

    SciTech Connect

    Kibler, M.; Smirnov, Yu. F.

    1995-03-05

    A purely group-theoretical approach (for which the symmetric group plays a central role), based upon the use of properties of fractional-parentage coefficients and isoscalar factors, is developed for the derivation of the Coulomb energy averaged over the states, with a definite spin, arising from an atomic configuration nl{sup N}. 15 refs.

  8. High Resolution Coherent Population Trapping on a Single Hole Spin in a Semiconductor Quantum Dot

    NASA Astrophysics Data System (ADS)

    Houel, Julien; Prechtel, Jonathan H.; Kuhlmann, Andreas V.; Brunner, Daniel; Kuklewicz, Christopher E.; Gerardot, Brian D.; Stoltz, Nick G.; Petroff, Pierre M.; Warburton, Richard J.

    2014-03-01

    We report high resolution coherent population trapping on a single hole spin in a semiconductor quantum dot. The absorption dip signifying the formation of a dark state exhibits an atomic physicslike dip width of just 10 MHz. We observe fluctuations in the absolute frequency of the absorption dip, evidence of very slow spin dephasing. We identify the cause of this process as charge noise by, first, demonstrating that the hole spin g factor in this configuration (in-plane magnetic field) is strongly dependent on the vertical electric field, and second, by characterizing the charge noise through its effects on the optical transition frequency. An important conclusion is that charge noise is an important hole spin dephasing process.

  9. New results on spin determination of nanosatellite BLITS from High Repetition Rate SLR data

    NASA Astrophysics Data System (ADS)

    Kucharski, D.; Kirchner, G.; Lim, H.-C.; Koidl, F.

    2013-03-01

    The nanosatellite BLITS (Ball Lens In The Space) demonstrates a successful design of the new spherical lens type satellite for Satellite Laser Ranging (SLR). The spin parameters of the satellite were calculated from more than 1000 days of SLR data collected from 6 High Repetition Rate (HRR) systems: Beijing, Changchun, Graz, Herstmonceux, Potsdam, Shanghai.Analysis of the 892 passes (September 26, 2009-June 18, 2012) shows precession of the spin axis around orientation of the along track vector calculated at the launch epoch of the satellite RA = 9h16m39s, Dec = 43.1°. The spin period of BLITS remains stable with the mean value Tmean = 5.613 s, RMS = 11 ms. The incident angle between the spin axis and the symmetry axis of the body changes within 60° range.

  10. Highly stable atomic vector magnetometer based on free spin precession.

    PubMed

    Afach, S; Ban, G; Bison, G; Bodek, K; Chowdhuri, Z; Grujić, Z D; Hayen, L; Hélaine, V; Kasprzak, M; Kirch, K; Knowles, P; Koch, H-C; Komposch, S; Kozela, A; Krempel, J; Lauss, B; Lefort, T; Lemière, Y; Mtchedlishvili, A; Naviliat-Cuncic, O; Piegsa, F M; Prashanth, P N; Quéméner, G; Rawlik, M; Ries, D; Roccia, S; Rozpedzik, D; Schmidt-Wellenburg, P; Severjins, N; Weis, A; Wursten, E; Wyszynski, G; Zejma, J; Zsigmond, G

    2015-08-24

    We present a magnetometer based on optically pumped Cs atoms that measures the magnitude and direction of a 1 μT magnetic field. Multiple circularly polarized laser beams were used to probe the free spin precession of the Cs atoms. The design was optimized for long-time stability and achieves a scalar resolution better than 300 fT for integration times ranging from 80 ms to 1000 s. The best scalar resolution of less than 80 fT was reached with integration times of 1.6 to 6 s. We were able to measure the magnetic field direction with a resolution better than 10 μrad for integration times from 10 s up to 2000 s. PMID:26368184

  11. Natural reference for nuclear high-spin states

    SciTech Connect

    Rowley, Neil; Ollier, James; Simpson, John

    2009-08-15

    We suggest two new representations of the data on rotational nuclei. The first is reference-free and the second arises from a natural reference related to the variable moment of inertia model parameters of the ground-state band of the system. As such, neither representation contains any free parameters. By defining a 'configuration spin' we show how a new ground-state band reference can be applied. Its use allows a complete description of the changes associated with the first, and higher, band crossings. We apply these new representations to discuss the nature of the first band crossing along even-even isotopic chains in the erbium and osmium isotopes and to odd-even nuclei in the vicinity of {sup 158}Er.

  12. High Energy Polarized e+e‑ Beams

    NASA Astrophysics Data System (ADS)

    Shatunov, Yu.; Koop, I.; Otboev, A.; Mane, S.

    2016-02-01

    Recently, the wide discussion about Higgs-factory design again returns to problem of high energy polarized electrons and positrons. It’s good known the radiative beam polarization at LEP-collider. It was obtained after spin resonance suppression at Z0 pick, but didn’t appear at energies above 70 GeV due to an enhancement of unavoidable depolarization effects. We examine in this paper various ideas for radiative polarization at TLEP/FCC-ee and formulate some estimates for the polarization buildup time and the asymptotic polarization. Using wigglers, a useful degree of polarization (for energy calibration), with a time constant of about 1 h, may be possible up to the threshold of W pair production. At higher energies such as the threshold of Higgs production, attaining a useful level of polarization may be difficult in a planar ring. With Siberian Snakes, wigglers and some imagination, polarization of reasonable magnitude, with a reasonable time constant (of not more than about 1 h), may be achievable at very high energies.

  13. Ultra high resolution neutron scattering: Neutron Resonance Spin-Echo and Larmor Diffraction

    NASA Astrophysics Data System (ADS)

    Walters, Andrew; Keller, Thomas; Keimer, Bernhard

    2012-02-01

    The TRISP spectrometer at the FRM II neutron source near Munich, Germany, is a unique world-leading neutron scattering instrument which employs the Neutron Resonance Spin-Echo technique (NRSE). Linewidths of dispersive excitations with energy transfers up to 50 meV can be measured with an energy resolution in the μeV range without the restrictive flux limitations that normally apply to high resolution neutron triple-axis spectrometers. Pioneering studies on the electron-phonon interaction in elemental superconductorsootnotetextP. Aynajian et al., Science 319 1509 (2008) and the lifetimes of magnetic excitations in archetypal magnetic systems will be reviewed.ootnotetextS. Bayrakci et al., Science 312 1928 (2006) The instrument can also be used as a Larmor diffractometer, enabling d-spacings to be measured with a resolution of δdd ˜10-6, i.e. more than one order of magnitude more sensitive than conventional diffraction techniques.ootnotetextC. Pfleiderer et al., Science 316 1871 (2007) Ongoing and future NRSE and Larmor diffraction projects will be outlined, especially in regard to prospective studies which will take full advantage of the new low temperature and high pressure sample environment capabilities now available at TRISP.

  14. High Energy Colliders

    NASA Astrophysics Data System (ADS)

    Palmer, R. B.; Gallardo, J. C.

    INTRODUCTION PHYSICS CONSIDERATIONS GENERAL REQUIRED LUMINOSITY FOR LEPTON COLLIDERS THE EFFECTIVE PHYSICS ENERGIES OF HADRON COLLIDERS HADRON-HADRON MACHINES LUMINOSITY SIZE AND COST CIRCULAR e^{+}e^- MACHINES LUMINOSITY SIZE AND COST e^{+}e^- LINEAR COLLIDERS LUMINOSITY CONVENTIONAL RF SUPERCONDUCTING RF AT HIGHER ENERGIES γ - γ COLLIDERS μ ^{+} μ^- COLLIDERS ADVANTAGES AND DISADVANTAGES DESIGN STUDIES STATUS AND REQUIRED R AND D COMPARISION OF MACHINES CONCLUSIONS DISCUSSION

  15. (High energy physics)

    SciTech Connect

    Bonner, B.E.; Roberts, J.B. Jr.

    1991-09-01

    An intense analysis effort on the data we obtained in a seven month run on E704 last year has produced a flood of new results on polarization effects in particle production at 200 GeV/c. We are fortunate to be able to report in detail on those results. Our other Fermilab experiment, E683 (photoproduction of jets) has been delayed an unbelievable amount of time by Fermilab schedule slippages. It was scheduled and ready for beam two years ago As this report is being written, we have been running for two months and are expecting four months of production data taking. In this report we show some of our preliminary results. In addition we are near the end of a six month run on our CERN experiment, NA47 (SMC) which will measure the spin dependent structure functions for the proton and neutron. It is with a sense of relief, mixed with pride, that we report that all the equipment which we constructed for that experiment is currently working as designed. The random coincidence of accelerator schedules has left us slightly dazed, but all experiments are getting done and analyzed in a timely fashion. As members of the Solenoidal Detector Collaboration, we have been preparing for the only currently approved experiment at the SSC. Here we report on our scintillating fiber tracker design and simulation activities. In addition we report the results of our investigation of the detector response to heavy Z particles. Since our last report, we have joined the D0 collaboration with the primary aim of contributing to the D0 upgrade over the next few years. It is also important for us to gain experience in collider physics during the period leading up to the SDC turn-on.

  16. Redox Thermodynamics of High-Spin and Low-Spin Forms of Chlorite Dismutases with Diverse Subunit and Oligomeric Structures

    PubMed Central

    2012-01-01

    Chlorite dismutases (Clds) are heme b-containing oxidoreductases that convert chlorite to chloride and dioxygen. In this work, the thermodynamics of the one-electron reduction of the ferric high-spin forms and of the six-coordinate low-spin cyanide adducts of the enzymes from Nitrobacter winogradskyi (NwCld) and Candidatus “Nitrospira defluvii” (NdCld) were determined through spectroelectrochemical experiments. These proteins belong to two phylogenetically separated lineages that differ in subunit (21.5 and 26 kDa, respectively) and oligomeric (dimeric and pentameric, respectively) structure but exhibit similar chlorite degradation activity. The E°′ values for free and cyanide-bound proteins were determined to be −119 and −397 mV for NwCld and −113 and −404 mV for NdCld, respectively (pH 7.0, 25 °C). Variable-temperature spectroelectrochemical experiments revealed that the oxidized state of both proteins is enthalpically stabilized. Molecular dynamics simulations suggest that changes in the protein structure are negligible, whereas solvent reorganization is mainly responsible for the increase in entropy during the redox reaction. Obtained data are discussed with respect to the known structures of the two Clds and the proposed reaction mechanism. PMID:23126649

  17. Energy transfer enhancement by oxygen perturbation of spin-forbidden electronic transitions in aromatic systems

    NASA Astrophysics Data System (ADS)

    Monguzzi, A.; Tubino, R.; Salamone, M. M.; Meinardi, F.

    2010-09-01

    Triplet-triplet energy transfer in multicomponent organic systems is usually entirely ascribed to a Dexter-type mechanism involving only short-range donor/acceptor interactions. We demonstrate that the presence of molecular oxygen introduces a perturbation to the electronic structure of one of the involved moieties which can induce a large increase in the spin-forbidden transition oscillator strength so that the otherwise negligible Förster contribution dominates the overall energy transfer rate.

  18. “Nodal Gap” induced by the incommensurate diagonal spin density modulation in underdoped high- Tc superconductors

    DOE PAGESBeta

    Zhou, Tao; Gao, Yi; Zhu, Jian -Xin

    2015-03-07

    Recenmore » tly it was revealed that the whole Fermi surface is fully gapped for several families of underdoped cuprates. The existence of the finite energy gap along the d-wave nodal lines (nodal gap) contrasts the common understanding of the d-wave pairing symmetry, which challenges the present theories for the high-Tcsuperconductors. Here we propose that the incommensurate diagonal spin-density-wave order can account for the above experimental observation. The Fermi surface and the local density of states are also studied. Our results are in good agreement with many important experiments in high-Tcsuperconductors.« less

  19. A High-Spin Rate Measurement Method for Projectiles Using a Magnetoresistive Sensor Based on Time-Frequency Domain Analysis.

    PubMed

    Shang, Jianyu; Deng, Zhihong; Fu, Mengyin; Wang, Shunting

    2016-01-01

    Traditional artillery guidance can significantly improve the attack accuracy and overall combat efficiency of projectiles, which makes it more adaptable to the information warfare of the future. Obviously, the accurate measurement of artillery spin rate, which has long been regarded as a daunting task, is the basis of precise guidance and control. Magnetoresistive (MR) sensors can be applied to spin rate measurement, especially in the high-spin and high-g projectile launch environment. In this paper, based on the theory of a MR sensor measuring spin rate, the mathematical relationship model between the frequency of MR sensor output and projectile spin rate was established through a fundamental derivation. By analyzing the characteristics of MR sensor output whose frequency varies with time, this paper proposed the Chirp z-Transform (CZT) time-frequency (TF) domain analysis method based on the rolling window of a Blackman window function (BCZT) which can accurately extract the projectile spin rate. To put it into practice, BCZT was applied to measure the spin rate of 155 mm artillery projectile. After extracting the spin rate, the impact that launch rotational angular velocity and aspect angle have on the extraction accuracy of the spin rate was analyzed. Simulation results show that the BCZT TF domain analysis method can effectively and accurately measure the projectile spin rate, especially in a high-spin and high-g projectile launch environment. PMID:27322266

  20. A High-Spin Rate Measurement Method for Projectiles Using a Magnetoresistive Sensor Based on Time-Frequency Domain Analysis

    PubMed Central

    Shang, Jianyu; Deng, Zhihong; Fu, Mengyin; Wang, Shunting

    2016-01-01

    Traditional artillery guidance can significantly improve the attack accuracy and overall combat efficiency of projectiles, which makes it more adaptable to the information warfare of the future. Obviously, the accurate measurement of artillery spin rate, which has long been regarded as a daunting task, is the basis of precise guidance and control. Magnetoresistive (MR) sensors can be applied to spin rate measurement, especially in the high-spin and high-g projectile launch environment. In this paper, based on the theory of a MR sensor measuring spin rate, the mathematical relationship model between the frequency of MR sensor output and projectile spin rate was established through a fundamental derivation. By analyzing the characteristics of MR sensor output whose frequency varies with time, this paper proposed the Chirp z-Transform (CZT) time-frequency (TF) domain analysis method based on the rolling window of a Blackman window function (BCZT) which can accurately extract the projectile spin rate. To put it into practice, BCZT was applied to measure the spin rate of 155 mm artillery projectile. After extracting the spin rate, the impact that launch rotational angular velocity and aspect angle have on the extraction accuracy of the spin rate was analyzed. Simulation results show that the BCZT TF domain analysis method can effectively and accurately measure the projectile spin rate, especially in a high-spin and high-g projectile launch environment. PMID:27322266

  1. Flare physics at high energies

    NASA Technical Reports Server (NTRS)

    Ramaty, R.

    1990-01-01

    High-energy processes, involving a rich variety of accelerated particle phenomena, lie at the core of the solar flare problem. The most direct manifestation of these processes are high-energy radiations, gamma rays, hard X-rays and neutrons, as well as the accelerated particles themselves, which can be detected in interplanetary space. In the study of astrophysics from the moon, the understanding of these processes should have great importance. The inner solar system environment is strongly influenced by activity on the sun; the physics of solar flares is of great intrinsic interest; and much high-energy astrophysics can be learned from investigations of flare physics at high energies.

  2. Nuclear spin polarization following intermediate-energy heavy-ion reactions

    SciTech Connect

    Groh, D. E.; Pinter, J. S.; Mantica, P. F.; Mertzimekis, T. J.; Stuchbery, A. E.; Khoa, D. T.

    2007-11-15

    Intermediate-energy heavy-ion collisions can produce a spin polarization of the projectile-like species. Spin polarization has been observed for both nucleon removal and nucleon pickup processes. Qualitative agreement with measured spin polarization as a function of the momentum of the projectile-like fragment is found in a kinematic model that considers conservation of linear and angular momentum and assumes peripheral interactions between the fast projectile and target. Better quantitative agreement was reached by including more realistic angular distributions and deorientation caused by {gamma}-ray emission and by correcting for the out-of-plane acceptance. The newly introduced corrections were found to apply to both nucleon removal and nucleon pickup processes.

  3. High-Spin States of {sup 84,85}Br: Mapping the Proton Sub-Shells towards {sup 78}Ni

    SciTech Connect

    Astier, A.; Porquet, M.-G.; Deloncle, I.; Venkova, Ts.; Azaiez, F.; Buta, A.; Curien, D.; Dorvaux, O.; Duchene, G.; Gall, B. J. P.; Khalfallah, F.; Piqueras, I.; Rousseau, M.; Meyer, M.; Redon, N.; Stezowski, O.; Lucas, R.

    2008-05-12

    The {sup 84,85}Br nuclei have been produced as fission fragments in the fusion reaction {sup 18}O+{sup 208}Pb at 85 MeV bombarding energy and studied with the Euroball IV array. The high-spin states of the odd-odd {sup 84}Br nucleus have been identified for the first time. From angular correlation analysis, spin values have been assigned to most of the {sup 85}Br excited states up to 4 MeV. All observed states in {sup 84,85}Br can be described by various proton excitations involving at least the two sub-shells ({pi}f{sub 5/2} and {pi}p{sub 3/2}) located just above the Z = 28 shell closure.

  4. Elastic energy and phase structure in a continuous spin Ising chain with applications to chiral homopolymers.

    PubMed

    Chernodub, M N; Lundgren, Martin; Niemi, Antti J

    2011-01-01

    We present a numerical Monte Carlo analysis of the phase structure in a continuous spin Ising chain that describes chiral homopolymers. We find that depending on the value of the Metropolis temperature, the model displays the three known nontrivial phases of polymers: At low temperatures the model is in a collapsed phase, at medium temperatures it is in a random walk phase, and at high temperatures it enters the self-avoiding random walk phase. By investigating the temperature dependence of the specific energy we confirm that the transition between the collapsed phase and the random walk phase is a phase transition, while the random walk phase and self-avoiding random walk phase are separated from each other by a crossover transition. We propose that the model can be applied to characterize the statistical properties of protein folding. For this we compare the predictions of the model to a phenomenological elastic energy formula, proposed by J. Lei and K. Huang [e-print arXiv:1002.5013; Europhys. Lett. 88, 68004 (2009)] to describe folded proteins. PMID:21405680

  5. Elastic energy and phase structure in a continuous spin Ising chain with applications to chiral homopolymers

    NASA Astrophysics Data System (ADS)

    Chernodub, M. N.; Lundgren, Martin; Niemi, Antti J.

    2011-01-01

    We present a numerical Monte Carlo analysis of the phase structure in a continuous spin Ising chain that describes chiral homopolymers. We find that depending on the value of the Metropolis temperature, the model displays the three known nontrivial phases of polymers: At low temperatures the model is in a collapsed phase, at medium temperatures it is in a random walk phase, and at high temperatures it enters the self-avoiding random walk phase. By investigating the temperature dependence of the specific energy we confirm that the transition between the collapsed phase and the random walk phase is a phase transition, while the random walk phase and self-avoiding random walk phase are separated from each other by a crossover transition. We propose that the model can be applied to characterize the statistical properties of protein folding. For this we compare the predictions of the model to a phenomenological elastic energy formula, proposed by J. Lei and K. Huang [e-print arXiv:1002.5013; Europhys. Lett.EULEEJ0295-507510.1209/0295-5075/88/68004 88, 68004 (2009)] to describe folded proteins.

  6. Possibilities of polarized protons in Sp anti p S and other high energy hadron colliders

    SciTech Connect

    Courant, E.D.

    1984-01-01

    The requirements for collisions with polarized protons in hadron colliders above 200 GeV are listed and briefly discussed. Particular attention is given to the use of the ''Siberan snake'' to eliminate depolarizing resonances, which occur when the spin precession frequency equals a frequency contained in the spectrum of the field seen by the beam. The Siberian snake is a device which makes the spin precession frequency essentially constant by using spin rotators, which precess the spin by 180/sup 0/ about either the longitudinal or transverse horizontal axis. It is concluded that operation with polarized protons should be possible at all the high energy hadron colliders. (LEW)

  7. QCD SPIN PHYSICS IN HADRONIC INTERACTIONS.

    SciTech Connect

    VOGELSANG,W.

    2007-06-19

    We discuss spin phenomena in high-energy hadronic scattering, with a particular emphasis on the spin physics program now underway at the first polarized proton-proton collider, RHIC. Experiments at RHIC unravel the spin structure of the nucleon in new ways. Prime goals are to determine the contribution of gluon spins to the proton spin, to elucidate the flavor structure of quark and antiquark polarizations in the nucleon, and to help clarify the origin of transverse-spin phenomena in QCD. These lectures describe some aspects of this program and of the associated physics.

  8. Quantized massive collective modes and massive spin fluctuations in high-Tc cuprates

    NASA Astrophysics Data System (ADS)

    Kanazawa, I.; Sasaki, T.

    2015-10-01

    We have analyzed angle-resolved photoemission spectra of the single- and double-layered Bi-family high-Tc superconductors by using quantized massive gauge fields, which might contain effects of spin fluctuations, charge fluctuations, and phonons. It is suggested strongly that the quantized massive gauge fields might be mediating Cooper pairing in high-Tc cuprates.

  9. Observation of a new high-spin isomer in {sup 94}Pd

    SciTech Connect

    Brock, T. S.; Nara Singh, B. S.; Wadsworth, R.; Boutachkov, P.; Gorska, M.; Grawe, H.; Pietri, S.; Domingo-Pardo, C.; Caceres, L.; Engert, T.; Farinon, F.; Gerl, J.; Goel, N.; Kojuharov, I.; Kurz, N.; Nociforo, C.; Prochazka, A.; Schaffner, H.; Weick, H.; Braun, N.

    2010-12-15

    A second {gamma}-decaying high-spin isomeric state, with a half-life of 197(22)ns, has been identified in the N=Z+2 nuclide {sup 94}Pd as part of a stopped-beam Rare Isotope Spectroscopic INvestigation at GSI (RISING) experiment. Weisskopf estimates were used to establish a tentative spin/parity of 19{sup -}, corresponding to the maximum possible spin of a negative parity state in the restricted (p{sub 1/2}, g{sub 9/2}) model space of empirical shell model calculations. The reproduction of the E3 decay properties of the isomer required an extension of the model space to include the f{sub 5/2} and p{sub 3/2} orbitals using the CD-Bonn potential. This is the first time that such an extension has been required for a high-spin isomer in the vicinity of {sup 100}Sn and reveals the importance of such orbits for understanding the decay properties of high-spin isomers in this region. However, despite the need for the extended model space for the E3 decay, the dominant configuration for the 19{sup -} state remains ({pi}p{sub 1/2}{sup -1}g{sub 9/2}{sup -3}){sub 11} x ({nu}g{sub 9/2}{sup -2}){sub 8}. The half-life of the known, 14{sup +}, isomer was remeasured and yielded a value of 499(13) ns.

  10. Evidence for single particle structure of high spin states in [sup 144]Pm and [sup 145]Pm

    SciTech Connect

    Glasmacher, T.; Caussyn, D.D.; Cottle, P.D.; Holcomb, J.W.; Johnson, T.D.; Kemper, K.W.; Kennedy, M.A.; Womble, P.C. )

    1993-06-01

    Excited states of the [ital Z]=61 isotopes [sup 144]Pm[sub 83] and [sup 154]Pm[sub 84] have been studied in the [sup 19]F+[sup 130]Te reaction at a beam energy of 85 MeV. Gamma-ray and conversion electron spectroscopy were used to establish the high spin states of [sup 144]Pm up to spin 20[h bar] and to extend the level spectrum of [sup 145]Pm up to a tentative spin of 33/2[h bar]. Empirical shell model calculations in a configuration space truncated to the [pi]1[ital h][sub 11/2], [pi]1[ital g][sub 7/2][sup [minus]1], and [pi]2[ital d][sub 5/2][sup [minus]1] protons and the [nu]2[ital f][sub 7/2] neutron outside the [sup 146]Gd core reproduce the observed energy levels in good agreement with the experimental results. ([pi][ital h][sub 11/2])[sup 2] configurations are suggested in an [ital N]=83 isotone for [ital Z][lt]64.

  11. High energy forming facility

    NASA Technical Reports Server (NTRS)

    Ciurlionis, B.

    1967-01-01

    Watertight, high-explosive forming facility, 25 feet in diameter and 15 feet deep, withstands repeated explosions of 10 pounds of TNT equivalent. The shell is fabricated of high strength steel and allows various structural elements to deform or move elastically and independently while retaining structural integrity.

  12. Quantum spin Hall insulator in halogenated arsenene films with sizable energy gaps

    PubMed Central

    Wang, Dongchao; Chen, Li; Shi, Changmin; Wang, Xiaoli; Cui, Guangliang; Zhang, Pinhua; Chen, Yeqing

    2016-01-01

    Based on first-principles calculations, the electronic and topological properties of halogenated (F-, Cl-, Br- and I-) arsenene are investigated in detail. It is found that the halogenated arsenene sheets show Dirac type characteristic in the absence of spin-orbital coupling (SOC), whereas energy gap will be induced by SOC with the values ranging from 0.194 eV for F-arsenene to 0.255 eV for I-arsenene. Noticeably, these four newly proposed two-dimensional (2D) systems are verified to be quantum spin Hall (QSH) insulators by calculating the edge states with obvious linear cross inside bulk energy gap. It should be pointed out that the large energy gap in these 2D materials consisted of commonly used element is quite promising for practical applications of QSH insulators at room temperature. PMID:27340091

  13. High energy nuclear collisions

    SciTech Connect

    Plasil, F.

    1998-01-01

    This presentation covers three broad topics: a brief introduction to the field of nucleus-nucleus collisions at relativistic energies; a discussion of several topics illustrating what`s been learned after more than a decade of fixed target experiments; and an indication of what the future may bring at the Relativistic Heavy Ion Collider (RHIC) under construction at the Brookhaven National Laboratory (BNL) and at the Large Hadron Collider (LHC) planned at CERN.

  14. The secondary coordination sphere controlled reactivity of a ferric-superoxo heme: unexpected conversion to a ferric hydroperoxo intermediate by reaction with a high-spin ferrous heme.

    PubMed

    Nagaraju, Perumandla; Ohta, Takehiro; Liu, Jin-Gang; Ogura, Takashi; Naruta, Yoshinori

    2016-06-01

    A bio-inspired heme complex involving both a proton donor and an axial imidazole ligand reduces the activation energy for the formation of a ferric hydroperoxo intermediate. A high-spin ferrous heme is shown to be capable of reducing its superoxy species to generate a ferric hydroperoxo intermediate for the first time. PMID:27105471

  15. Dynamical effects of spin-dependent interactions in low- and intermediate-energy heavy-ion reactions

    NASA Astrophysics Data System (ADS)

    Xu, Jun; Li, Bao-An; Shen, Wen-Qing; Xia, Yin

    2015-10-01

    It is well known that noncentral nuclear forces, such as the spin-orbital coupling and the tensor force, play important roles in understanding many interesting features of nuclear structures. However, their dynamical effects in nuclear reactions are poorly known because only the spin-averaged observables are normally studied both experimentally and theoretically. Realizing that spin-sensitive observables in nuclear reactions may convey useful information about the in-medium properties of noncentral nuclear interactions, besides earlier studies using the time-dependent Hartree-Fock approach to understand the effects of spin-orbital coupling on the threshold energy and spin polarization in fusion reactions, some efforts have been made recently to explore the dynamical effects of noncentral nuclear forces in intermediate-energy heavy-ion collisions using transport models. The focus of these studies has been on investigating signatures of the density and isospin dependence of the form factor in the spin-dependent single-nucleon potential. Interestingly, some useful probes were identified in the model studies but so far there are still no data to compare with. In this brief review, we summarize the main physics motivations as well as the recent progress in understanding the spin dynamics and identifying spin-sensitive observables in heavy-ion reactions at intermediate energies. We hope the interesting, important, and new physics potentials identified in the spin dynamics of heavy-ion collisions will stimulate more experimental work in this direction.

  16. High-spin states in the N=50 nucleus ^87Rb

    NASA Astrophysics Data System (ADS)

    Fotiades, N.; Cizewski, J. A.; Krücken, R.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Becker, J. A.; Bernstein, L. A.; McNabb, D. P.; Younes, W.

    2001-10-01

    High-spin states in ^87Rb have been studied following the fission of two compound nuclei (^199Tl and ^197Pb) formed in different fusion-evaporation reactions. The Gammasphere array at LBNL was used to detect γ-ray coincidences. The level scheme has been extended above the previously known 1578 keV, 9/2^+ isomer by observation of many states up to ~7.2 MeV excitation energy. Coupling of the odd g_9/2 proton to the yrast states in the ^86Kr core accounts for the first excited states observed above the 9/2^+ isomer. The level scheme of ^87Rb is also compared to excitations in ^85Kr and the ^89Y isotone. This work has been supported in part by the U.S. Department of Energy under Contracts No. W-7405-ENG-36 (LANL), FG02-91ER-40609 (Yale), W-7405-ENG-48 (LLNL) and AC03-76SF00098 (LBNL) and by the National Science Foundation (Rutgers).

  17. High-Spin Structures in the N = 153 Nucleus 251Cf

    NASA Astrophysics Data System (ADS)

    Qiu, Y.; Hota, S. S.; Chowdhury, P.; Guess, C. J.; Jackson, E. G.; Lister, C. J.; Prasher, V. S.; Khoo, T. L.; Carpenter, M. P.; Janssens, R. V. F.; Greene, J.; Ahmad, I.; Seweryniak, D.; Zhu, S.; Albers, M.; Alcorta, M.; Bertone, P. F.; Chen, J.; Chiara, C. J.; Hoffman, C. R.; Kondev, F. G.; Lauritsen, T.; Tandel, S. K.

    2013-10-01

    In continuation of our exploration of band structures in neutron-rich Cf nuclei using inelastic and transfer reactions, we report new spectroscopic observations in the 251Cf nucleus. High-spin states of neutron-rich Cf nuclei were populated using a 208Pb beam from the ATLAS facility at Argonne, incident on a radioactive target mixture of 249 , 250 , 251Cf. Prompt γ rays were detected by the Gammasphere array. Both signatures of the ground state band of 251Cf were observed for the first time, with enhanced signal-to-noise achieved through appropriate gates on sum energy and fold parameters. Assignment of the band structure to 251Cf is via coincidence with Cf X-rays as well as the excitation of the 208Pb beam partner. Configurations are assigned to the observed band from experimental M1/E2 branching ratios from clean decays within the band. Further data analysis is in progress, and the new results will be discussed in the context of physics of the highest neutron orbitals accessible to spectroscopy in the A = 250 region. Work supported by U.S. Department of Energy.

  18. In-beam studies of high-spin states of actinide nuclei

    SciTech Connect

    Stoyer, M.A. . Nuclear Science Div. California Univ., Berkeley, CA . Dept. of Chemistry)

    1990-11-15

    High-spin states in the actinides have been studied using Coulomb- excitation, inelastic excitation reactions, and one-neutron transfer reactions. Experimental data are presented for states in {sup 232}U, {sup 233}U, {sup 234}U, {sup 235}U, {sup 238}Pu and {sup 239}Pu from a variety of reactions. Energy levels, moments-of-inertia, aligned angular momentum, Routhians, gamma-ray intensities, and cross-sections are presented for most cases. Additional spectroscopic information (magnetic moments, M{sub 1}/E{sub 2} mixing ratios, and g-factors) is presented for {sup 233}U. One- and two-neutron transfer reaction mechanisms and the possibility of band crossings (backbending) are discussed. A discussion of odd-A band fitting and Cranking calculations is presented to aid in the interpretation of rotational energy levels and alignment. In addition, several theoretical calculations of rotational populations for inelastic excitation and neutron transfer are compared to the data. Intratheory comparisons between the Sudden Approximation, Semi-Classical, and Alder-Winther-DeBoer methods are made. In connection with the theory development, the possible signature for the nuclear SQUID effect is discussed. 98 refs., 61 figs., 21 tabs.

  19. Calculations with the quasirelativistic local-spin-density-functional theory for high-Z atoms

    SciTech Connect

    Guo, Y.; Whitehead, M.A.

    1988-10-01

    The generalized-exchange local-spin-density-functional theory (LSD-GX) with relativistic corrections of the mass velocity and Darwin terms has been used to calculate statistical total energies for the neutral atoms, the positive ions, and the negative ions for high-Z elements. The effect of the correlation and relaxation correction on the statistical total energy is discussed. Comparing the calculated results for the ionization potentials and electron affinities for the atoms (atomic number Z from 37 to 56 and 72 to 80) with experiment, shows that for the atoms rubidium to barium both the LSD-GX and the quasirelativistic LSD-GX, with self-interaction correction, Gopinathan, Whitehead, and Bogdanovic's Fermi-hole parameters (Phys. Rev. A 14, 1 (1976)), and Vosko, Wilk, and Nusair's correlation correction (Can. J. Phys. 58, 1200 (1980)), are very good methods for calculating ionization potentials and electron affinities. For the atoms hafnium to mercury the relativistic effect has to be considered.

  20. High Energy Flywheel Containment Evaluation

    NASA Technical Reports Server (NTRS)

    Colozza, Anthony J.; Trase, Larry (Technical Monitor)

    2000-01-01

    A flywheel testing facility is being constructed at the NASA Glenn Research Center. This facility is to be used for life cycle testing of various flywheel rotors. The lifecycle testing consists of spinning a rotor from a low rpm (approx. 20,000 ) to a high rpm (approx. 60,000) and then back to the low rpm. This spin cycle will model that which the rotor will see during use. To simulate the lifetime of the rotor, the spin cycle will be performed tens of thousands of times. A typical life cycle spin test is expected to last six months. During this time the rotor will be spun through a cycle every five minutes. The test will run continuously for the six month period barring a flywheel failure. Since it is not reasonable to have the surrounding area evacuated of personnel for the duration of the testing, the flywheel facility has to be designed to withstand a flywheel rotor failure and insure that there is no danger to any personnel in the adjacent buildings or surrounding areas. In order to determine if the facility can safely contain a flywheel rotor failure an analysis of the facility in conjunction with possible flywheel failure modes was performed. This analysis is intended as a worst case evaluation of the burst liner and vacuum tank's ability to contain a failure. The test chamber consists of a cylindrical stainless steel vacuum tank, two outer steel containment rings, and a stainless steel burst liner. The stainless steel used is annealed 302, which has an ultimate strength of 620 MPa (90,000 psi). A diagram of the vacuum tank configuration is shown. The vacuum tank and air turbine will be located below ground in a pit. The tank is secured in the pit with 0.3 m (12 in.) of cement along the base and the remaining portion of the tank is surrounded by gravel up to the access ports. A 590 kg (1300 lb.) bulkhead is placed on top of the pit during operation and the complete facility is housed within a concrete structure which has 7.5 cm (3 in.) thick walls. A cutaway

  1. Impact on Spin Tune From Horizontal Orbital Angle Between Snakes and Orbital Angle Between Spin Rotators

    SciTech Connect

    Bai,M.; Ptitsyn, V.; Roser, T.

    2008-10-01

    To keep the spin tune in the spin depolarizing resonance free region is required for accelerating polarized protons to high energy. In RHIC, two snakes are located at the opposite side of each accelerator. They are configured to yield a spin tune of 1/2. Two pairs of spin rotators are located at either side of two detectors in each ring in RHIC to provide longitudinal polarization for the experiments. Since the spin rotation from vertical to longitudinal is localized between the two rotators, the spin rotators do not change the spin tune. However, due to the imperfection of the orbits around the snakes and rotators, the spin tune can be shifted. This note presents the impact of the horizontal orbital angle between the two snakes on the spin tune, as well as the effect of the vertical orbital angle between two rotators at either side of the collision point on the spin tune.

  2. High resolution x-ray fluorescence spectroscopy - a new technique for site- and spin-selectivity

    SciTech Connect

    Wang, Xin

    1996-12-01

    X-ray spectroscopy has long been used to elucidate electronic and structural information of molecules. One of the weaknesses of x-ray absorption is its sensitivity to all of the atoms of a particular element in a sample. Through out this thesis, a new technique for enhancing the site- and spin-selectivity of the x-ray absorption has been developed. By high resolution fluorescence detection, the chemical sensitivity of K emission spectra can be used to identify oxidation and spin states; it can also be used to facilitate site-selective X-ray Absorption Near Edge Structure (XANES) and site-selective Extended X-ray Absorption Fine Structure (EXAFS). The spin polarization in K fluorescence could be used to generate spin selective XANES or spin-polarized EXAFS, which provides a new measure of the spin density, or the nature of magnetic neighboring atoms. Finally, dramatic line-sharpening effects by the combination of absorption and emission processes allow observation of structure that is normally unobservable. All these unique characters can enormously simplify a complex x-ray spectrum. Applications of this novel technique have generated information from various transition-metal model compounds to metalloproteins. The absorption and emission spectra by high resolution fluorescence detection are interdependent. The ligand field multiplet model has been used for the analysis of K{alpha} and K{beta} emission spectra. First demonstration on different chemical states of Fe compounds has shown the applicability of site selectivity and spin polarization. Different interatomic distances of the same element in different chemical forms have been detected using site-selective EXAFS.

  3. Ab initio study of the influence of structural parameters on the potential energy surfaces of spin-crossover Fe(II) model compounds

    NASA Astrophysics Data System (ADS)

    Boilleau, Corentin; Suaud, Nicolas; Guihéry, Nathalie

    2012-12-01

    In spin-crossover (SCO) compounds exhibiting a light induced excited spin state trapping (LIESST) effect, the thermodynamic T1/2 and kinetic T(LIESST) temperature values depend on the features of the potential energy surfaces (PES) of the two lowest singlet and quintet states but also on vibrational contributions, collective effects, such as electrostatics, for instance, spin-orbit couplings to a lesser extent, etc. In this work, the question of the link between the shape of the PES of SCO compounds exhibiting a LIESST effect and their first coordination sphere structure is addressed from wave function theory based ab initio calculations. Fe(II) complexes based on model ligands suited to reproduce the main characteristics of the PES of such compounds are distorted to emphasize selectively the role played by the metal-ligand distances and the ligand-metal-ligand angles. The studied angular deformations are those usually observed in many Fe(L)2(NCS)2 complexes. It is shown that the larger the deformation between the low spin and high spin equilibrium geometries, the higher the energy barrier from the high spin state and the weaker the energy difference between the bottom of the wells. These results corroborate observations made by experimentalists on a large number of complexes. While the PES features only constitutes one of the contributions to these temperatures, it is worth noticing that, relating T1/2 to the energy difference between the bottoms of the singlet and quintet wells and the T(LIESST) to the energy barrier from the quintet bottom well, the same slope of the empirical law T(LIESST) = -0.3T1/2+T0 is observed.

  4. Rotor Design for High Pressure Magic Angle Spinning Nuclear Magnetic Resonance

    SciTech Connect

    Turcu, Romulus V.F.; Hoyt, David W.; Rosso, Kevin M.; Sears, Jesse A.; Loring, John S.; Felmy, Andrew R.; Hu, Jian Z.

    2013-01-01

    High pressure magic angle spinning (MAS) nuclear magnetic resonance (NMR) with a sample spinning rate exceeding 2.1 kHz and pressure greater than 165 bar has never been realized. In this work, a new sample cell design is reported, suitable for constructing cells of different sizes. Using a 7.5 mm high pressure MAS rotor as an example, internal pressure as high as 200 bar at a sample spinning rate of 6 kHz is achieved. The new high pressure MAS rotor is re-usable and compatible with most commercial NMR set-ups, exhibiting low 1H and 13C NMR background and offering maximal NMR sensitivity. As an example of its many possible applications, this new capability is applied to determine reaction products associated with the carbonation reaction of a natural mineral, antigorite ((Mg,Fe2+)3Si2O5(OH)4), in contact with liquid water in water-saturated supercritical CO2 (scCO2) at 150 bar and 50 deg C. This mineral is relevant to the deep geologic disposal of CO2, but its iron content results in too many sample spinning sidebands at low spinning rate. Hence, this chemical system is a good case study to demonstrate the utility of the higher sample spinning rates that can be achieved by our new rotor design. We expect this new capability will be useful for exploring solid-state, including interfacial, chemistry at new levels of high-pressure in a wide variety of fields.

  5. Rotor design for high pressure magic angle spinning nuclear magnetic resonance.

    PubMed

    Turcu, Romulus V F; Hoyt, David W; Rosso, Kevin M; Sears, Jesse A; Loring, John S; Felmy, Andrew R; Hu, Jian Zhi

    2013-01-01

    High pressure magic angle spinning (MAS) nuclear magnetic resonance (NMR) with a sample spinning rate exceeding 2.1 kHz and pressure greater than 165 bar has never been realized. In this work, a new sample cell design is reported, suitable for constructing cells of different sizes. Using a 7.5 mm high pressure MAS rotor as an example, internal pressure as high as 200 bar at a sample spinning rate of 6 kHz is achieved. The new high pressure MAS rotor is re-usable and compatible with most commercial NMR set-ups, exhibiting low (1)H and (13)C NMR background and offering maximal NMR sensitivity. As an example of its many possible applications, this new capability is applied to determine reaction products associated with the carbonation reaction of a natural mineral, antigorite ((Mg,Fe(2+))(3)Si(2)O(5)(OH)(4)), in contact with liquid water in water-saturated supercritical CO(2) (scCO(2)) at 150 bar and 50°C. This mineral is relevant to the deep geologic disposal of CO(2), but its iron content results in too many sample spinning sidebands at low spinning rate. Hence, this chemical system is a good case study to demonstrate the utility of the higher sample spinning rates that can be achieved by our new rotor design. We expect this new capability will be useful for exploring solid-state, including interfacial, chemistry at new levels of high-pressure in a wide variety of fields. PMID:23220181

  6. Rotor design for high pressure magic angle spinning nuclear magnetic resonance

    NASA Astrophysics Data System (ADS)

    Turcu, Romulus V. F.; Hoyt, David W.; Rosso, Kevin M.; Sears, Jesse A.; Loring, John S.; Felmy, Andrew R.; Hu, Jian Zhi

    2013-01-01

    High pressure magic angle spinning (MAS) nuclear magnetic resonance (NMR) with a sample spinning rate exceeding 2.1 kHz and pressure greater than 165 bar has never been realized. In this work, a new sample cell design is reported, suitable for constructing cells of different sizes. Using a 7.5 mm high pressure MAS rotor as an example, internal pressure as high as 200 bar at a sample spinning rate of 6 kHz is achieved. The new high pressure MAS rotor is re-usable and compatible with most commercial NMR set-ups, exhibiting low 1H and 13C NMR background and offering maximal NMR sensitivity. As an example of its many possible applications, this new capability is applied to determine reaction products associated with the carbonation reaction of a natural mineral, antigorite ((Mg,Fe2+)3Si2O5(OH)4), in contact with liquid water in water-saturated supercritical CO2 (scCO2) at 150 bar and 50 °C. This mineral is relevant to the deep geologic disposal of CO2, but its iron content results in too many sample spinning sidebands at low spinning rate. Hence, this chemical system is a good case study to demonstrate the utility of the higher sample spinning rates that can be achieved by our new rotor design. We expect this new capability will be useful for exploring solid-state, including interfacial, chemistry at new levels of high-pressure in a wide variety of fields.

  7. Spin wave excitations in low-energy electron scattering off Fe surfaces

    NASA Astrophysics Data System (ADS)

    Vernoy, Michael; Hopster, Herbert

    2002-03-01

    For the last two decades, SPEELS has been instrumental in the investigation of Stoner excitations in ferromagnets. By analyzing the spin of both the scattered electron beam and the incident beam, so called “complete” experiments were performed [1,2]. By eliminating the spin analysis of the scattered beam it has become possible to examine short wavelength spin wave excitations [3]. We constructed a 127 degree cylindrical deflector spectrometer with an analyzer rotatable to 70 degrees. The polarized electron beam is produced by a negative electron affinity GaAs photocathode. Initial data were taken with a primary beam energy of 20 V at a resolution of 50 meV FWHM on thick Fe/GaAs films. Spin asymmetries show the Stoner continuum as noted in the previous complete experiments as well as an additional feature in the 100-300 meV energy loss region. Angle dependent data will be presented. [1] J. Kirschner, Phys. Rev. Lett. 55, 973 (1985). [2] D. L. Abraham and H. Hopster, Phys. Rev. Lett. 59, 2333 (1987). [3] M. Plihal, D. L. Mills, and J. Kirschner, Phys. Rev. Lett. 82, 2579 (1999).

  8. High-fidelity transfer and storage of photon states in a single nuclear spin

    NASA Astrophysics Data System (ADS)

    Yang, Sen; Wang, Ya; Rao, D. D. Bhaktavatsala; Hien Tran, Thai; Momenzadeh, Ali S.; Markham, M.; Twitchen, D. J.; Wang, Ping; Yang, Wen; Stöhr, Rainer; Neumann, Philipp; Kosaka, Hideo; Wrachtrup, Jörg

    2016-08-01

    Long-distance quantum communication requires photons and quantum nodes that comprise qubits for interaction with light and good memory capabilities, as well as processing qubits for the storage and manipulation of photons. Owing to the unavoidable photon losses, robust quantum communication over lossy transmission channels requires quantum repeater networks. A necessary and highly demanding prerequisite for these networks is the existence of quantum memories with long coherence times to reliably store the incident photon states. Here we demonstrate the high-fidelity (∼98%) coherent transfer of a photon polarization state to a single solid-state nuclear spin that has a coherence time of over 10 s. The storage process is achieved by coherently transferring the polarization state of a photon to an entangled electron–nuclear spin state of a nitrogen–vacancy centre in diamond. The nuclear spin-based optical quantum memory demonstrated here paves the way towards an absorption-based quantum repeater network.

  9. High domain wall velocities via spin transfer torque using vertical current injection

    PubMed Central

    Metaxas, Peter J.; Sampaio, Joao; Chanthbouala, André; Matsumoto, Rie; Anane, Abdelmadjid; Fert, Albert; Zvezdin, Konstantin A.; Yakushiji, Kay; Kubota, Hitoshi; Fukushima, Akio; Yuasa, Shinji; Nishimura, Kazumasa; Nagamine, Yoshinori; Maehara, Hiroki; Tsunekawa, Koji; Cros, Vincent; Grollier, Julie

    2013-01-01

    Domain walls, nanoscale transition regions separating oppositely oriented ferromagnetic domains, have significant promise for use in spintronic devices for data storage and memristive applications. The state of these devices is related to the wall position and thus rapid operation will require a controllable onset of domain wall motion and high speed wall displacement. These processes are traditionally driven by spin transfer torque due to lateral injection of spin polarized current through a ferromagnetic nanostrip. However, this geometry is often hampered by low maximum wall velocities and/or a need for prohibitively high current densities. Here, using time-resolved magnetotransport measurements, we show that vertical injection of spin currents through a magnetic tunnel junction can drive domain walls over hundreds of nanometers at ~500 m/s using current densities on the order of 6 MA/cm2. Moreover, these measurements provide information about the stochastic and deterministic aspects of current driven domain wall mediated switching. PMID:23670402

  10. High domain wall velocities via spin transfer torque using vertical current injection.

    PubMed

    Metaxas, Peter J; Sampaio, Joao; Chanthbouala, André; Matsumoto, Rie; Anane, Abdelmadjid; Fert, Albert; Zvezdin, Konstantin A; Yakushiji, Kay; Kubota, Hitoshi; Fukushima, Akio; Yuasa, Shinji; Nishimura, Kazumasa; Nagamine, Yoshinori; Maehara, Hiroki; Tsunekawa, Koji; Cros, Vincent; Grollier, Julie

    2013-01-01

    Domain walls, nanoscale transition regions separating oppositely oriented ferromagnetic domains, have significant promise for use in spintronic devices for data storage and memristive applications. The state of these devices is related to the wall position and thus rapid operation will require a controllable onset of domain wall motion and high speed wall displacement. These processes are traditionally driven by spin transfer torque due to lateral injection of spin polarized current through a ferromagnetic nanostrip. However, this geometry is often hampered by low maximum wall velocities and/or a need for prohibitively high current densities. Here, using time-resolved magnetotransport measurements, we show that vertical injection of spin currents through a magnetic tunnel junction can drive domain walls over hundreds of nanometers at ~500 m/s using current densities on the order of 6 MA/cm(2). Moreover, these measurements provide information about the stochastic and deterministic aspects of current driven domain wall mediated switching. PMID:23670402

  11. High domain wall velocities via spin transfer torque using vertical current injection

    NASA Astrophysics Data System (ADS)

    Metaxas, Peter J.; Sampaio, Joao; Chanthbouala, André; Matsumoto, Rie; Anane, Abdelmadjid; Fert, Albert; Zvezdin, Konstantin A.; Yakushiji, Kay; Kubota, Hitoshi; Fukushima, Akio; Yuasa, Shinji; Nishimura, Kazumasa; Nagamine, Yoshinori; Maehara, Hiroki; Tsunekawa, Koji; Cros, Vincent; Grollier, Julie

    2013-05-01

    Domain walls, nanoscale transition regions separating oppositely oriented ferromagnetic domains, have significant promise for use in spintronic devices for data storage and memristive applications. The state of these devices is related to the wall position and thus rapid operation will require a controllable onset of domain wall motion and high speed wall displacement. These processes are traditionally driven by spin transfer torque due to lateral injection of spin polarized current through a ferromagnetic nanostrip. However, this geometry is often hampered by low maximum wall velocities and/or a need for prohibitively high current densities. Here, using time-resolved magnetotransport measurements, we show that vertical injection of spin currents through a magnetic tunnel junction can drive domain walls over hundreds of nanometers at ~500 m/s using current densities on the order of 6 MA/cm2. Moreover, these measurements provide information about the stochastic and deterministic aspects of current driven domain wall mediated switching.

  12. Exchange Coupling Inversion in a High-Spin Organic Triradical Molecule.

    PubMed

    Gaudenzi, R; Burzurí, E; Reta, D; Moreira, I de P R; Bromley, S T; Rovira, C; Veciana, J; van der Zant, H S J

    2016-03-01

    The magnetic properties of a nanoscale system are inextricably linked to its local environment. In adatoms on surfaces and inorganic layered structures, the exchange interactions result from the relative lattice positions, layer thicknesses, and other environmental parameters. Here, we report on a sample-dependent sign inversion of the magnetic exchange coupling between the three unpaired spins of an organic triradical molecule embedded in a three-terminal device. This ferro-to-antiferromagnetic transition is due to structural distortions and results in a high-to-low spin ground-state change in a molecule traditionally considered to be a robust high-spin quartet. Moreover, the flexibility of the molecule yields an in situ electric tunability of the exchange coupling via the gate electrode. These findings open a route to the controlled reversal of the magnetic states in organic molecule-based nanodevices by mechanical means, electrical gating, or chemical tailoring. PMID:26862681

  13. Non-collective high-spin states in /sup 148/Dy

    SciTech Connect

    Dines, E.L.

    1985-04-01

    General physical concepts regarding nuclear high-spin states are given. The high-spin states in /sup 148/Dy(Z = 66, N = 82) were produced via the reaction /sup 112/Cd(Pb-backed)(/sup 40/Ar,4n) at E/sub lab/ = 175, at the 88-inch Cyclotron at Lawrence Berkeley Laboratory. Methods for placing gates on various transitions above and below the 480 nsec isomer at 10/sup +/(known from previous work), as well as for calculating transition intensities and their associated errors, are given. Calculations of angular correlations for multiple ..gamma..-ray cascades, assuming non-zero-width distributions in m-states for some given spin state, were done and compared to experimental values. Analysis of RF - Ge and Ge - Ge TAC spectra for transitions above the 480 nsec isomer implied lifetimes of less than or equal to 5 nsec (except for the 327.2 keV transition). Using such analysis, some 19 new ..gamma..-ray transitions were discovered above the isomer, thereby extending the /sup 148/Dy level scheme up to spin I = 31 h-bar. Assignments of spins and parities for the new levels are made based on information obtained from angular correlations and the lifetime limits. Previous work on the 11 transitions below the 480 nsec isomer is confirmed.

  14. Effect of transverse vibrations of fissile nuclei on the angular and spin distributions of low-energy fission fragments

    NASA Astrophysics Data System (ADS)

    Bunakov, V. E.; Kadmensky, S. G.; Lyubashevsky, D. E.

    2016-05-01

    It is shown that A. Bohr's classic theory of angular distributions of fragments originating from low-energy fission should be supplemented with quantum corrections based on the involvement of a superposition of a very large number of angular momenta L m in the description of the relative motion of fragments flying apart along the straight line coincidentwith the symmetry axis. It is revealed that quantum zero-point wriggling-type vibrations of the fissile system in the vicinity of its scission point are a source of these angular momenta and of high fragment spins observed experimentally.

  15. High-spin isomers in 212Rn in the region of triple neutron core-excitations

    NASA Astrophysics Data System (ADS)

    Dracoulis, G. D.; Lane, G. J.; Byrne, A. P.; Davidson, P. M.; Kibédi, T.; Nieminen, P.; Watanabe, H.; Wilson, A. N.

    2008-04-01

    The level scheme of 212Rn has been extended to spins of ∼ 38 ℏ and excitation energies of about 13 MeV using the 204Hg(13C, 5n)212Rn reaction and γ-ray spectroscopy. Time correlated techniques have been used to obtain sensitivity to weak transitions and channel selectivity. The excitation energy of the 22+ core-excited isomer has been established at 6174 keV. Two isomers with τ = 25 (2) ns and τ = 12 (2) ns are identified at 12211 and 12548 keV, respectively. These are the highest-spin nuclear isomers now known, and are attributed to configurations involving triple neutron core-excitations coupled to the aligned valence protons. Semi-empirical shell-model calculations can account for most states observed, but with significant energy discrepancies for some configurations.

  16. Single crystal diffraction studies of phase transition of minerals across Fe high-low spin transition at high pressure

    NASA Astrophysics Data System (ADS)

    Merlini, M.; Hanfland, M.

    2011-12-01

    The spin state of Fe in structure of minerals relevant for the lower mantle mineralogy, is known to undergo a high to low spin state change. This phenomena is often coupled to a remarkable volume contraction and from a structural point of view, often is associated to isosymmetrical phase transition. Recent improvements at X-Ray beamlines for diffraction at extreme conditions at synchrotron facilities allow the possibility to perform single crystal diffraction and determine crystal structure of minerals at extreme conditions, including also structural studies across first or second order phase transition. The accurate knowledge of crystal structure and of phase behaviour at high pressure is a very important step in order to: 1-understand the physical properties; 2- have an accurate experimental constraint on numerical simulation. We report here three examples of structure determination by single crystal X-Ray diffraction at extreme conditions concerning phase transition related to Fe spin state change, measured at ID09A beamline (ESRF, France). CaFe2O4 undergoes a spin transition at 50 GPa. XRD before and after indicate the symmetry and crystal structure is the same. The transition is marked by 10 % volume contraction. The use of He as pressure transmitting media strongly reduced strain induced by pressure and let the crystal survive this transition, allowing for the first time direct determination of Fe-O bond length changes related to variation of spin state. The main structural difference between high and low spin structure is simply a collapse of FeO6 polyhedra. FeCO3 has been also investigated, and the results are also compared with already present in literature. FeCO3 undergoes a transition around 45 GPa, with a remarked hysteresis. In the pressure range 20-45 however an anomalous behaviour is noticed, probably related to a different spin interaction due to reduced Fe-Fe distances. Fe1-xS pyrrhotite has been investigated in two different structure (a

  17. High-spin states in the semimagic nucleus 89Y and neutron-core excitations in the N =50 isotones

    NASA Astrophysics Data System (ADS)

    Li, Z. Q.; Wang, S. Y.; Niu, C. Y.; Qi, B.; Wang, S.; Sun, D. P.; Liu, C.; Xu, C. J.; Liu, L.; Zhang, P.; Wu, X. G.; Li, G. S.; He, C. Y.; Zheng, Y.; Li, C. B.; Yu, B. B.; Hu, S. P.; Yao, S. H.; Cao, X. P.; Wang, J. L.

    2016-07-01

    The semimagic nucleus 89Y 89 has been investigated using the 82Se(11>B,4 n ) reaction at beam energies of 48 and 52 MeV. More than 24 new transitions have been identified, leading to a considerable extension of the level structures of 89Y. The experimental results are compared with the large-basis shell model calculations. They show that cross-shell neutron excitations play a pivotal role in high-spin level structures of 89Y. The systematic features of neutron-core excitations in the N =50 isotones are also discussed.

  18. 34. mu. s isomer at high spin in sup 212 Fr: Evidence for a many-particle octupole coupled state

    SciTech Connect

    Byrne, A.P.; Dracoulis, G.D.; Schiffer, K.J.; Davidson, P.M.; Kibedi, T.; Fabricius, B.; Baxter, A.M.; Stuchbery, A.E. Australian National University, G.P.O. Box 4, Canberra, Australian Capital Territory )

    1990-07-01

    A very high spin isomeric state with {tau}{sub {ital m}}=34(3) {mu}s has been observed at an excitation energy of 8.5 MeV in {sup 212}Fr. The experimental evidence favors an {ital E}3 assignment, with a very large {ital E}3 transition strength, {ital B}({ital E}3)=100(12){times}10{sup 3} {ital e}{sup 2}fm{sup 6}, to one of the {gamma} rays de-exciting the isomer. The observed properties are in very good agreement with the characteristics of a 34{sup +} state predicted by the multiparticle octupole vibration model.

  19. The straintronic spin-neuron.

    PubMed

    Biswas, Ayan K; Atulasimha, Jayasimha; Bandyopadhyay, Supriyo

    2015-07-17

    In artificial neural networks, neurons are usually implemented with highly dissipative CMOS-based operational amplifiers. A more energy-efficient implementation is a 'spin-neuron' realized with a magneto-tunneling junction (MTJ) that is switched with a spin-polarized current (representing weighted sum of input currents) that either delivers a spin transfer torque or induces domain wall motion in the soft layer of the MTJ to mimic neuron firing. Here, we propose and analyze a different type of spin-neuron in which the soft layer of the MTJ is switched with mechanical strain generated by a voltage (representing weighted sum of input voltages) and term it straintronic spin-neuron. It dissipates orders of magnitude less energy in threshold operations than the traditional current-driven spin neuron at 0 K temperature and may even be faster. We have also studied the room-temperature firing behaviors of both types of spin neurons and find that thermal noise degrades the performance of both types, but the current-driven type is degraded much more than the straintronic type if both are optimized for maximum energy-efficiency. On the other hand, if both are designed to have the same level of thermal degradation, then the current-driven version will dissipate orders of magnitude more energy than the straintronic version. Thus, the straintronic spin-neuron is superior to current-driven spin neurons. PMID:26112081

  20. Low-energy singlet excitations in spin-1/2 Heisenberg antiferromagnet on square lattice

    NASA Astrophysics Data System (ADS)

    Aktersky, A. Yu.; Syromyatnikov, A. V.

    2016-05-01

    We present an approach based on a dimer expansion which describes low-energy singlet excitations (singlons) in spin-1/2 Heisenberg antiferromagnet on simple square lattice. An operator ("effective Hamiltonian") is constructed whose eigenvalues give the singlon spectrum. The "effective Hamiltonian" looks like a Hamiltonian of a spin-1/2 magnet in strong external magnetic field and it has a gapped spectrum. It is found that singlet states lie above triplet ones (magnons) in the whole Brillouin zone except in the vicinity of the point (π , 0), where their energies are slightly smaller. Based on this finding, we suggest that a magnon decay is possible near (π , 0) into another magnon and a singlon which may contribute to the dip of the magnon spectrum near (π , 0) and reduce the magnon lifetime. It is pointed out that the singlon-magnon continuum may contribute to the continuum of excitations observed recently near (π , 0).

  1. Quantum energy teleportation across a three-spin Ising chain in a Gibbs state

    NASA Astrophysics Data System (ADS)

    Trevison, Jose; Hotta, Masahiro

    2015-05-01

    In general, it is important to identify what is the informational resource for quantum tasks. Quantum energy teleportation (QET) is a quantum task, which attains energy transfer in an operational sense by local operations and classical communication, and is expected to play a role in future development of nano-scale smart grids. We consider QET protocols in a three-element Ising spin system with non-periodic boundary conditions coupled to a thermal bath. The open chain is the minimal model of QET between two edge spins that allows the measurement and operation steps of the QET protocol to be optimized without restriction. It is possible to analyze how two-body correlations of the system, such as mutual information, entanglement and quantum discord, can be resources of this QET at each temperature. In particular, we stress that quantum discord is not the QET resource in some cases, even if arbitrary measurements and operations are available.

  2. Spectral spin diffusion and magnetic dipolar energy in the NMR of 13CH3 compounds.

    PubMed

    Ylinen, E E; Kankaanpää, M; Punkkinen, M

    2006-06-01

    Spin diffusion between 13CH3 groups in solids is studied both theoretically and experimentally. It is shown to be dominated by mutual spin flip-flops of protons belonging to neighbouring methyl groups. Also nonmethyl protons may contribute significantly if present in the sample. The spin-rotational ground state of 13CH3 consists of 16 sublevels. When their populations are used to describe spin diffusion, eight population combinations are shown to be important, two of them corresponding to the 13C-proton and proton-proton intra-methyl magnetic dipolar energies, Dc and Dp, respectively. Spin-diffusion transitions modulate these combinations so that a further reduction to two sets of four combinations is possible, with no coupling between the sets. Coupled differential equations are derived to describe the time dependence of the combinations in each set. They are solved numerically and compared with experimental results on a single crystal of aspirin with 13C-labelled methyl groups at the carbon resonance. The 13C NMR induction signal was observed as a function of time after the preparation either at the carbon resonance (a two-pulse sequence) or at the proton resonance (proton saturation). Usually carbon spectra were computed first and then three of the mentioned population combinations were obtained from the individual spectral components. Some results on the time dependence of Dc were also obtained directly from the amplitude of the out-of-phase induction signal. Theoretical predictions are found to describe semiquantitatively the overall time dependence of these three combinations and especially their variation with different initial conditions, which are discussed in detail. Also the partial transfer of the magnetic dipolar energy between Dc and Dp is nicely explained. Reasons for discrepancies are discussed. PMID:16361090

  3. Novel spin-on organic hardmask with high plasma etch resistance

    NASA Astrophysics Data System (ADS)

    Oh, Chang-Il; Lee, Jin-Kuk; Kim, Min-Soo; Yoon, Kyong-Ho; Cheon, Hwan-Sung; Tokareva, Nataliya; Song, Jee-Yun; Kim, Jong-Seob; Chang, Tu-Won

    2008-03-01

    In recent years for memory devices under 70nm using ArF lithography, spin-on organic hardmask has become an attractive alternative process to amorphous carbon layer hardmark (ACL) in mass production due to ACL hardmask's limited capacity, high cost-of-ownership, and low process efficiency in spite of its excellent etch performance. However, insufficient plasma etch resistance of spin-on hardmask makes the etch process an issue resulting in inadequate vertical profiles, large CD bias, and narrow etch process window compared to ACL hardmask. In order to be able to apply these spin on hardmasks to varies layers including critical layers, the aforementioned problems need to be resolved and verified using several evaluation methods including etch pattern evaluation. In this paper, we report the synthesis of novel organic spin-on hardmasks (C-SOH) that incorporate various fused aromatic moieties into polymer chain and the evaluation of etch performance using dry etch tools. Organic spin-on hardmasks with 79-90 wt% carbon contents were synthesized in-house. Oxygen and fluorine based plasma etch processes were used to evaluate the etch resistance of the C-SOH. The results show our 3rd generation C-SOH has etch profiles comparable to that of ACL in a 1:1 dense pattern.

  4. Giant spin-driven ferroelectric polarization in TbMnO3 under high pressure.

    PubMed

    Aoyama, T; Yamauchi, K; Iyama, A; Picozzi, S; Shimizu, K; Kimura, T

    2014-01-01

    The recent research on multiferroics has provided solid evidence that the breaking of inversion symmetry by spin order can induce ferroelectric polarization P. This type of multiferroics, called spin-driven ferroelectrics, often show a gigantic change in P on application of a magnetic field B. However, their polarization (<~0.1 μC cm(-2)) is much smaller than that in conventional ferroelectrics (typically several to several tens of μC cm(-2)). Here we show that the application of external pressure to a representative spin-driven ferroelectric, TbMnO3, causes a flop of P and leads to the highest P (≈ 1.0 μC cm(-2)) among spin-driven ferroelectrics ever reported. We explain this behaviour in terms of a pressure-induced magnetoelectric phase transition, based on the results of density functional simulations. In the high-pressure phase, the application of B further enhances P over 1.8 μC cm(-2). This value is nearly an order of magnitude larger than those ever reported in spin-driven ferroelectrics. PMID:25215855

  5. Experimental High Energy Neutrino Astrophysics

    SciTech Connect

    Distefano, Carla

    2005-10-12

    Neutrinos are considered promising probes for high energy astrophysics. More than four decades after deep water Cerenkov technique was proposed to detect high energy neutrinos. Two detectors of this type are successfully taking data: BAIKAL and AMANDA. They have demonstrated the feasibility of the high energy neutrino detection and have set first constraints on TeV neutrino production astrophysical models. The quest for the construction of km3 size detectors have already started: in the South Pole, the IceCube neutrino telescope is under construction; the ANTARES, NEMO and NESTOR Collaborations are working towards the installation of a neutrino telescope in the Mediterranean Sea.

  6. High-energy spectroscopic astrophysics

    NASA Astrophysics Data System (ADS)

    Güdel, Manuel; Walter, Roland

    After three decades of intense research in X-ray and gamma-ray astronomy, the time was ripe to summarize basic knowledge on X-ray and gamma-ray spectroscopy for interested students and researchers ready to become involved in new high-energy missions. This volume exposes both the scientific basics and modern methods of high-energy spectroscopic astrophysics. The emphasis is on physical principles and observing methods rather than a discussion of particular classes of high-energy objects, but many examples and new results are included in the three chapters as well.

  7. High Spin States and Octupole Deformation in Neutron-Rich ^145,147La Nuclei

    NASA Astrophysics Data System (ADS)

    Zhu, S. J.; Hamilton, J. H.; Ramayya, A. V.; Babu, B. R. S.; Jones, E. F.; Kormicki, J.; Daniel, A. V.; Hwang, J. K.; Beyer, C. J.; Wang, M. G.; Long, G. L.; Li, M.; Zhu, L. Y.; Gan, C. Y.; Ma, W. C.; Cole, J. D.; Aryaeinejad, R.; Dardenne, Y. X.; Drigert, M. W.; Rasmussen, J. O.; Asztalos, S.; Lee, I. Y.; Macchiavelli, A. O.; Chu, S. Y.; Gregorich, K. E.; Mohar, M. F.; Stoyer, M. A.; Lougheed, R. W.; Moody, K. J.; Wild, J. F.; Prussin, S. G.

    1998-04-01

    High spin states in neutron-rich odd-Z nuclei ^145,147La have been investigated from the study of prompt γ- rays in spontaneous fission of ^252Cf by using γ-γ- and γ-γ-γ- coincidence techniques. Alternating parity bands are extended up to spins I=(41/2) and I=(43/2) in ^145La and ^147La, respectively. Strong E1 transitions between the negative and positive parity bands give evidence for stable octupole deformation. The new higher spin levels give evidence for rotational enhancement of the stability of the octupole deformation. These collective bands show competition and co-existence between symmetric and asymmetric shapes in ^145La. Band crossing was found around hbarω≈ 0.26 ~0.30 MeV in both nuclei and these backbends are related to the alignment of two i_13/2 neutron from cranked shell model calculations.

  8. Spin crossover in Fe2SiO4 liquid at high pressure

    NASA Astrophysics Data System (ADS)

    Ramo, David Muñoz; Stixrude, Lars

    2014-07-01

    We combine spin-polarized density functional theory with first principle molecular dynamics (FPMD) to study the spin crossover in liquid Fe2SiO4, up to 300 GPa and 6000 K. In contrast to the much sharper transition seen in crystals, we find that the high- to low-spin transition occurs over a very broad pressure interval (>200 GPa) due to structural disorder in the liquid. We find excellent agreement with the experimental Hugoniot. We combine our results with previous FPMD calculations to derive the partial molar volumes of the oxide components MgO, FeO, and SiO2. We find that eutectic melts in the MgO-FeO-SiO2 system are denser than coexisting solids in the bottom 600 km of Earth's mantle.

  9. High spin polarization in CoFeMnGe equiatomic quaternary Heusler alloy

    SciTech Connect

    Bainsla, Lakhan; Suresh, K. G.; Nigam, A. K.; Manivel Raja, M.; Varaprasad, B. S. D. Ch. S.; Takahashi, Y. K.; Hono, K.

    2014-11-28

    We report the structure, magnetic property, and spin polarization of CoFeMnGe equiatomic quaternary Heusler alloy. The alloy was found to crystallize in the cubic Heusler structure (prototype LiMgPdSn) with considerable amount of DO{sub 3} disorder. Thermal analysis result indicated the Curie temperature is about 750 K without any other phase transformation up to melting temperature. The magnetization value was close to that predicted by the Slater-Pauling curve. Current spin polarization of P = 0.70 ± 0.01 was deduced using point contact andreev reflection measurements. The temperature dependence of electrical resistivity has been fitted in the temperature range of 5–300 K in order to check for the half metallic behavior. Considering the high spin polarization and Curie temperature, this material appears to be promising for spintronic applications.

  10. Unexpected Spin-Crossover and a Low-Pressure Phase Change in an Iron(II)/Dipyrazolylpyridine Complex Exhibiting a High-Spin Jahn- Teller Distortion.

    PubMed

    Kershaw Cook, Laurence J; Thorp-Greenwood, Flora L; Comyn, Tim P; Cespedes, Oscar; Chastanet, Guillaume; Halcrow, Malcolm A

    2015-07-01

    The synthesis of 4-methyl-2,6-di(pyrazol-1-yl)pyridine (L) and four salts of [FeL2]X2 (X– = BF(4)(–), 1; X– = ClO(4)(–), 2; X– = PF(6)(–), 3; X– = CF3SO(3)(–), 4) are reported. Powder samples of 1 and 2 both exhibit abrupt, hysteretic spin-state transitions on cooling, with T(1/2)↓ = 204 and T(1/2)↑ = 209 K (1), and T(1/2)↓ = 175 and T(1/2)↑ = 193 K (2). The 18 K thermal hysteresis loop for 2 is unusually wide for a complex of this type. Single crystal structures of 2 show it to exhibit a Jahn–Teller-distorted six-coordinate geometry in its high-spin state, which would normally inhibit spin-crossover. Bulk samples of 1 and 2 are isostructural by X-ray powder diffraction, and undergo a crystallographic phase change during their spin-transitions. At temperatures below T(1/2), exposing both compounds to 10(–5) Torr pressure inside the powder diffractometer causes a reversible transformation back to the high-temperature crystal phase. Consideration of thermodynamic data implies this cannot be accompanied by a low → high spin-state change, however. Both compounds also exhibit the LIESST effect, with 2 exhibiting an unusually high T(LIESST) of 112 K. The salts 3 and 4 are respectively high-spin and low-spin between 3 and 300 K, with crystalline 3 exhibiting a more pronounced version of the same Jahn–Teller distortion. PMID:26351707

  11. Unexpected Spin-Crossover and a Low-Pressure Phase Change in an Iron(II)/Dipyrazolylpyridine Complex Exhibiting a High-Spin Jahn-Teller Distortion.

    PubMed

    Kershaw Cook, Laurence J; Thorp-Greenwood, Flora L; Comyn, Tim P; Cespedes, Oscar; Chastanet, Guillaume; Halcrow, Malcolm A

    2015-07-01

    The synthesis of 4-methyl-2,6-di(pyrazol-1-yl)pyridine (L) and four salts of [FeL2]X2 (X(-) = BF4(-), 1; X(-) = ClO4(-), 2; X(-) = PF6(-), 3; X(-) = CF3SO3(-), 4) are reported. Powder samples of 1 and 2 both exhibit abrupt, hysteretic spin-state transitions on cooling, with T1/2↓ = 204 and T1/2↑ = 209 K (1), and T1/2↓ = 175 and T1/2↑ = 193 K (2). The 18 K thermal hysteresis loop for 2 is unusually wide for a complex of this type. Single crystal structures of 2 show it to exhibit a Jahn-Teller-distorted six-coordinate geometry in its high-spin state, which would normally inhibit spin-crossover. Bulk samples of 1 and 2 are isostructural by X-ray powder diffraction, and undergo a crystallographic phase change during their spin-transitions. At temperatures below T1/2, exposing both compounds to 10(-5) Torr pressure inside the powder diffractometer causes a reversible transformation back to the high-temperature crystal phase. Consideration of thermodynamic data implies this cannot be accompanied by a low → high spin-state change, however. Both compounds also exhibit the LIESST effect, with 2 exhibiting an unusually high T(LIESST) of 112 K. The salts 3 and 4 are respectively high-spin and low-spin between 3 and 300 K, with crystalline 3 exhibiting a more pronounced version of the same Jahn-Teller distortion. PMID:26052980

  12. High energy physics

    SciTech Connect

    Kernan, A.; Shen, B.C.; Ma, E.

    1997-07-01

    Hadron collider studies will focus on: (i) the search for the top quark with the newly installed D0 detector at the Fermilab Tevatron collider, (ii) the upgrade of the D0 detector to match the new main injector luminosity and (iii) R&D on silicon microstrip tracking devices for the SSC. High statistics studies of Z{sup 0} decay will continue with the OPAL detector at LEP. These studies will include a direct measurement of Z decay to neutrinos, the search for Higgs and heavy quark decays of Z. Preparations for the Large Scintillation Neutrino Detector (LSND) to measure neutrino oscillations at LAMPF will focus on data acquisition and testing of photomultiplier tubes. In the theoretical area E. Ma will concentrate on mass-generating radiative mechanisms for light quarks and leptons in renormalizable gauge field theories. J. Wudka`s program includes a detailed investigation of the magnetic-flip approach to the solar neutrino.

  13. Free-energy analysis of spin models on hyperbolic lattice geometries

    NASA Astrophysics Data System (ADS)

    Serina, Marcel; Genzor, Jozef; Lee, Yoju; Gendiar, Andrej

    2016-04-01

    We investigate relations between spatial properties of the free energy and the radius of Gaussian curvature of the underlying curved lattice geometries. For this purpose we derive recurrence relations for the analysis of the free energy normalized per lattice site of various multistate spin models in the thermal equilibrium on distinct non-Euclidean surface lattices of the infinite sizes. Whereas the free energy is calculated numerically by means of the corner transfer matrix renormalization group algorithm, the radius of curvature has an analytic expression. Two tasks are considered in this work. First, we search for such a lattice geometry, which minimizes the free energy per site. We conjecture that the only Euclidean flat geometry results in the minimal free energy per site regardless of the spin model. Second, the relations among the free energy, the radius of curvature, and the phase transition temperatures are analyzed. We found out that both the free energy and the phase transition temperature inherit the structure of the lattice geometry and asymptotically approach the profile of the Gaussian radius of curvature. This achievement opens new perspectives in the AdS-CFT correspondence theories.

  14. Intermediate/high energy nuclear physics. [Iowa State Univ. , Ames, Iowa

    SciTech Connect

    Vary, J.P.

    1992-01-01

    Progress during the last year is reviewed under the following topics: relativistic hadron--nucleus and nucleus--nucleus collisions (heavy meson production, photon production and fragmentation functions--direct photon production with the QCM and photon fragmentation functions, Cronin efffect and multiple scattering, effective nuclear parton distributions); solving quantum field theories in nonperturbative regime; light-front dynamics and high-spin states (soft form factor of the pion and nucleon for transverse and longitudinal momentum transfers, light front spinors for high-spin objects); high-energy spin physics; relativistic wave equations, quarkonia, and e[sup +]e[sup [minus

  15. Future of high energy physics

    SciTech Connect

    Panofsky, W.K.H.

    1984-06-01

    A rough overview is given of the expectations for the extension of high energy colliders and accelerators into the xtremely high energy range. It appears likely that the SSC or something like it will be the last gasp of the conventional method of producing high energy proton-proton collisions using synchrotron rings with superconducting magnets. It is likely that LEP will be the highest energy e+e/sup -/ colliding beam storage ring built. The future beyond that depends on the successful demonstrations of new technologies. The linear collider offers hope in this respect for some extension in energy for electrons, and maybe even for protons, but is too early to judge whether, by how much, or when such an extension will indeed take place.

  16. Energy input and HI spin temperatures in low pressure regions

    NASA Technical Reports Server (NTRS)

    Corbelli, E.; Salpeter, E. E.

    1990-01-01

    Two recent (unpublished) HI emission/absorption studies carried out with good sensitivity using the Arecibo 21 cm beam are discussed. One study (Colgan, Salpeter and Terzian) looked for high velocity clouds of our own Galaxy in absorption in the directions of 63 of the brightest continuum sources reachable with the Arecibo telescope. HI emission mapping in the neighborhood of these directions was also carried out. The other study (Corbelli and Schneider) looked for absorption along lines of sight to about 50 weaker sources which pass within a few diameters of nearby disk galaxies. Neither study detected any absorption.

  17. High energy physics

    SciTech Connect

    Not Available

    1992-04-10

    The Counter Group continues to work on data analysis for Fermilab Experiment E653. Altogether, they expect several thousand reconstructed charm events and approximately 25 B pair events of which 12 have been observed thus far. Preparation continue for Fermilab Experiment E781, a high statistics study of charm baryon production. In the Theory Group, Cutkosky and collaborators study hadron phenomenology and non-perturbative QCD calculations. Levine has a long standing program in computational QED to obtain improved theoretical values for g-2 of the electron. Wolfenstein, Li, and their collaborators have worked on areas of weak interaction phenomenology that may yield insights beyond the standard model, e.g. CP violation and non-zero neutrino masses. Holman has been concerned with phase transitions in gauge theories relevant to cosmological problems. During 1991 most of the group effort was concentrated on the L3 experiment at CERN. Highlights of the results from the analysis of the Z[degrees] resonance include (a) a measurement of the strong coupling constant [alpha][sub s] for b quarks (b) a precision measurement of the average time of B hadrons and (c) a direct determination of the number of light neutrino faculties from the reaction e[sup +]e[sup [minus

  18. Perturbational treatment of spin-orbit coupling for generally applicable high-level multi-reference methods

    SciTech Connect

    Mai, Sebastian; Marquetand, Philipp; González, Leticia; Müller, Thomas; Plasser, Felix; Lischka, Hans

    2014-08-21

    An efficient perturbational treatment of spin-orbit coupling within the framework of high-level multi-reference techniques has been implemented in the most recent version of the COLUMBUS quantum chemistry package, extending the existing fully variational two-component (2c) multi-reference configuration interaction singles and doubles (MRCISD) method. The proposed scheme follows related implementations of quasi-degenerate perturbation theory (QDPT) model space techniques. Our model space is built either from uncontracted, large-scale scalar relativistic MRCISD wavefunctions or based on the scalar-relativistic solutions of the linear-response-theory-based multi-configurational averaged quadratic coupled cluster method (LRT-MRAQCC). The latter approach allows for a consistent, approximatively size-consistent and size-extensive treatment of spin-orbit coupling. The approach is described in detail and compared to a number of related techniques. The inherent accuracy of the QDPT approach is validated by comparing cuts of the potential energy surfaces of acrolein and its S, Se, and Te analoga with the corresponding data obtained from matching fully variational spin-orbit MRCISD calculations. The conceptual availability of approximate analytic gradients with respect to geometrical displacements is an attractive feature of the 2c-QDPT-MRCISD and 2c-QDPT-LRT-MRAQCC methods for structure optimization and ab inito molecular dynamics simulations.

  19. High energy physics

    SciTech Connect

    Not Available

    1992-04-10

    The Counter Group continues to work on data analysis for Fermilab Experiment E653. Altogether, they expect several thousand reconstructed charm events and approximately 25 B pair events of which 12 have been observed thus far. Preparation continue for Fermilab Experiment E781, a high statistics study of charm baryon production. In the Theory Group, Cutkosky and collaborators study hadron phenomenology and non-perturbative QCD calculations. Levine has a long standing program in computational QED to obtain improved theoretical values for g-2 of the electron. Wolfenstein, Li, and their collaborators have worked on areas of weak interaction phenomenology that may yield insights beyond the standard model, e.g. CP violation and non-zero neutrino masses. Holman has been concerned with phase transitions in gauge theories relevant to cosmological problems. During 1991 most of the group effort was concentrated on the L3 experiment at CERN. Highlights of the results from the analysis of the Z{degrees} resonance include (a) a measurement of the strong coupling constant {alpha}{sub s} for b quarks (b) a precision measurement of the average time of B hadrons and (c) a direct determination of the number of light neutrino faculties from the reaction e{sup +}e{sup {minus}} {yields} {nu}{bar {nu}}{gamma}. We also began a major upgrade of the L3 luminosity monitor by replacing PWC chamber by a Si strip system in front of the BGO calorimeters. Finally we have continued our SSC R&D work on BaF{sub 2} by joining the GEM collaboration.

  20. Energy spectra of high energy atmospheric neutrinos

    NASA Technical Reports Server (NTRS)

    Mitsui, K.; Minorikawa, Y.

    1985-01-01

    Focusing on high energy neutrinos ( or = 1 TeV), a new calculation of atmospheric neutrino intensities was carried out taking into account EMC effects observed in P-A collisions by accelerator, recent measurement of primary cosmic ray spectrum and results of cosmic ray muon spectrum and charge ratio. Other features of the present calculation are (1) taking into account kinematics of three body decays of kaons and charm particles in diffusion equations and (2) taking into account energy dependence of kaon production.

  1. Dipole bands in high spin states of {sub 57}{sup 135}La{sub 78}

    SciTech Connect

    Garg, Ritika; Kumar, S.; Saxena, Mansi; Goyal, Savi; Siwal, Davinder; Verma, S.; Mandal, S.; Palit, R.; Saha, Sudipta; Sethi, J.; Sharma, Sushil K.; Trivedi, T.; Jadav, S. K.; Donthi, R.; Naidu, B. S.

    2014-08-14

    High spin states of {sup 135}La have been investigated using the reaction {sup 128}Te({sup 11}B,4n){sup 135}La at a beam energy of 50.5 MeV. Two negative parity dipole bands (ΔI = 1) have been established. Crossover E2 transitions have been observed for the first time in one of the dipole bands. For the Tilted Axis Cranking (TAC) calculations, a three-quasiparticle (3qp) configuration π(h{sub 11/2}){sup 1}⊗ν(h{sub 11/2}){sup −2} and a five-quasiparticle (5qp) configuration π(h{sub 11/2}){sup 1}(g{sub 7/2}/d{sub 5/2}){sup 2}⊗ν(h{sub 11/2}){sup −2} have been taken for the two negative parity dipole bands. The comparison of experimental observables with TAC calculations supports the configuration assignments for both the dipole bands.

  2. High spin states in {sup 151,153}Pr, {sup 157}Sm, and {sup 93}Kr

    SciTech Connect

    Hwang, J. K.; Ramayya, A. V.; Hamilton, J. H.; Liu, S. H.; Brewer, N. T.; Luo, Y. X.; Rasmussen, J. O.; Zhu, S. J.; Donangelo, R.

    2010-09-15

    High spin states are observed for the first time in the neutron-rich nuclei {sup 151,153}Pr, {sup 157}Sm, and {sup 93}Kr from the spontaneous fission of {sup 252}Cf. Twenty new transitions in {sup 151}Pr, twelve in {sup 153}Pr, five in {sup 157}Sm, and four in {sup 93}Kr were identified by using x-ray(Pr/Sm)-{gamma}-{gamma} and {gamma}-{gamma}-{gamma} triple coincidences. From the measured total internal conversion coefficients {alpha}{sub T} of four low-energy transitions in {sup 151,153}Pr, we determine that two bands in each nucleus have opposite parity. The interlacing E1 transitions between the bands suggest a form of parity doubling in {sup 151,153}Pr. New bands in {sup 157}Sm and {sup 93}Kr are reported. The half-life of the 354.8 keV state in {sup 93}Kr is measured to be 10(2) ns.

  3. Excess energy and decoherence factor of a qubit coupled to a one-dimensional periodically driven spin chain

    NASA Astrophysics Data System (ADS)

    Nag, Tanay

    2016-06-01

    We take a central spin model (CSM), consisting of a one-dimensional environmental Ising spin chain and a single qubit connected globally to all the spins of the environment, to study the excess energy (EE) of the environment and the logarithm of decoherence factor namely, generalized fidelity susceptibility per site (GFSS), associated with the qubit under a periodic driving of the transverse field term of environment across its critical point using the Floquet theory. The coupling to the qubit, prepared in a pure state, with the transverse field of the spin chain yields two sets of EE corresponding to the two species of Floquet operators. In the limit of weak coupling, we derive an approximated expression of GFSS after an infinite number of driving period which can successfully estimate the low- and intermediate-frequency behavior of GFSS obtained numerically with a large number of time periods. Our main focus is to analytically investigate the effect of system-environment coupling strength on the EEs and GFSS and relate the behavior of GFSS to EEs as a function of frequency by plausible analytical arguments. We explicitly show that the low-frequency beatinglike pattern of GFSS is an outcome of two frequencies, causing the oscillations in the two branches of EEs, that are dependent on the coupling strength. In the intermediate frequency regime, dip structure observed in GFSS can be justified by the resonance peaks of EEs at those coupling parameter-dependent frequencies; high-frequency saturation behavior of EEs and GFSS are controlled by the same static Hamiltonian and the associated saturation values are related to the coupling strength.

  4. Investigation of high-spin states in 53Fe

    SciTech Connect

    du Rietz, R.; Williams, S.J.; Rudolph, D.; Ekman, J.; Fahlander,C.; Andreoiu, C.; Axiotis, M.; Bentley, M.A.; Carpenter, M.P.; Chandler,C.; Charity, R.J.; Clark, R.M.; Cromaz, M.; Dewald, A.; de Angelis, G.; Della Vedova, F.; Fallon, P.; Gadea, A.; Hammond, G.; Ideguchi, E.; Lenzi, S.M.; Macchiavelli, A.O.; Marginean, N.; Mineva, M.N.; Moller, O.; DNapoli, .R.; Nespolo, M.; Reviol, W.; Rusu, C.; Saha, B.; Sarantites,D.G.; Seweryniak, D.; Tonev, D.; Ur, C.A.

    2006-04-15

    The fusion-evaporation reactions 28Si(32S,1{alpha}2p1n)53Fe at 125 MeV and 24Mg(32S,2p1n)53Fe at a 95-MeV beam energy were used to investigate excited states in 53Fe. The combination of the Gammasphere Ge detector array and ancillary devices led to the construction of an extensive level scheme comprising some 90 transitions connecting 40 states. The lifetime of the yrast 25/2- state and upper limits for the lifetimes of a number of additional states were determined using the Cologne plunger device coupled to the GASP {gamma}-ray spectrometer. The experimental results are compared to large-scale shell-model calculations using different sets of two-body matrix elements. In particular, predictions on electromagnetic decay properties such as lifetimes, branching ratios, and mixing ratios are studied in detail.

  5. Fusion with highly spin polarized HD and D sub 2

    SciTech Connect

    Honig, A. . Dept. of Physics); Kremens, R.; Skupsky, S. . Lab. for Laser Energetics)

    1991-05-05

    During the course of this grant, we succeeded in overcoming essentially all of the obstacles on the route to carrying out ICF shots with polarized deuteron fuel in plastic target shells. ICF with polarized deuterons is expected to answer the question of survival of polarization in the high temperature plasma prior to fusion, as well as to give quantitative information on anisotropic particle emissions and possible suppression of particular fusion reactions. The techniques previously developed for high D polarization in large solid HD samples have been adapted to polystyrene target shells which are cooled conductively via very thin metal wire supports. An independent NMR experiment on a normal-D{sub 2}-filled glass target shell with 2 {mu}m copper-coated spider silk supports affirmed the thermal conduction adequacy by registering very low sample temperatures in the presence of the generation of considerable D{sub 2} conversion heat. In a permeation experiment employing very pure ortho-D{sub 2}, it was demonstrated that hydrogens diffuse into polystyrene shells at room temperature without molecular dissociation, a requirement for preservation of the composition of our HD samples used for polarization. An advanced version of the permeation apparatus was designed and constructed which permits preparation of target shells loaded with very high density HD or D{sub 2} fuels. That system includes provision for cryocondensation and cold-transfer either to the dilution refrigerator for polarization or to the OMEGA fusion chamber for ICF experiments with denser unpolarized fuel targets than were heretofore realizable in plastic target shells. a major effort resulted in improvements of cold-transfer inter-apparatus mating procedures which minimize the temperature rise of the target shells over that of the helium reservoir temperature. High D polarization in solid pure 0-D{sub 2} was shown to be retained into the liquid state after rapid melting.

  6. Multidomain Human Peroxidasin 1 Is a Highly Glycosylated and Stable Homotrimeric High Spin Ferric Peroxidase*

    PubMed Central

    Soudi, Monika; Paumann-Page, Martina; Delporte, Cedric; Pirker, Katharina F.; Bellei, Marzia; Edenhofer, Eva; Stadlmayr, Gerhard; Battistuzzi, Gianantonio; Boudjeltia, Karim Zouaoui; Furtmüller, Paul G.; Van Antwerpen, Pierre; Obinger, Christian

    2015-01-01

    Human peroxidasin 1 (hsPxd01) is a multidomain heme peroxidase that uses bromide as a cofactor for the formation of sulfilimine cross-links. The latter confers critical structural reinforcement to collagen IV scaffolds. Here, hsPxd01 and various truncated variants lacking nonenzymatic domains were recombinantly expressed in HEK cell lines. The N-glycosylation site occupancy and disulfide pattern, the oligomeric structure, and unfolding pathway are reported. The homotrimeric iron protein contains a covalently bound ferric high spin heme per subunit with a standard reduction potential of the Fe(III)/Fe(II) couple of −233 ± 5 mV at pH 7.0. Despite sequence homology at the active site and biophysical properties similar to human peroxidases, the catalytic efficiency of bromide oxidation (kcat/KMapp) of full-length hsPxd01 is rather low but increased upon truncation. This is discussed with respect to its structure and proposed biosynthetic function in collagen IV cross-linking. PMID:25713063

  7. NMR spectroscopy of hyperpolarized ^129Xe at high fields: Maintaining spin polarization after optical pumping.

    NASA Astrophysics Data System (ADS)

    Patton, Brian; Kuzma, Nicholas N.; Lisitza, Natalia V.; Happer, William

    2003-05-01

    Spin-polarized ^129Xe has become an invaluable tool in nuclear magnetic resonance research, with applications ranging from medical imaging to high-resolution spectroscopy. High-field NMR studies using hyperpolarized xenon as a spectroscopic probe benefit from the high signal-to-noise ratios and large chemical shifts typical of optically-pumped noble gases. The experimental sensitivity is ultimately determined by the absolute polarization of the xenon in the sample, which can be substantially decreased during purification and transfer. NMR of xenon at high fields (9.4 Tesla) will be discussed, and potential mechanisms of spin relaxation during the distillation, storage(N. N. Kuzma, B. Patton, K. Raman, and W. Happer, Phys. Rev. Lett. 88), 147602 (2002)., and delivery of hyperpolarized xenon will be analyzed.

  8. Investigation of high-spin states in {sup 53}Fe

    SciTech Connect

    Rietz, R. du; Rudolph, D.; Ekman, J.; Fahlander, C.; Andreoiu, C.; Mineva, M.N.; Williams, S.J.; Bentley, M.A.; Chandler, C.; Hammond, G.; Axiotis, M.; De Angelis, G.; Gadea, A.; Marginean, N.; Napoli, D. R.; Nespolo, M.; Rusu, C.; Tonev, D.; Ur, C.A.; Carpenter, M.P.

    2005-07-01

    The fusion-evaporation reactions {sup 28}Si({sup 32}S,1{alpha}2p1n){sup 53}Fe at 125 MeV and {sup 24}Mg({sup 32}S,2p1n){sup 53}Fe at a 95-MeV beam energy were used to investigate excited states in {sup 53}Fe. The combination of the Gammasphere Ge detector array and ancillary devices led to the construction of an extensive level scheme comprising some 90 transitions connecting 40 states. The lifetime of the yrast 25/2{sup -} state and upper limits for the lifetimes of a number of additional states were determined using the Cologne plunger device coupled to the GASP {gamma}-ray spectrometer. The experimental results are compared to large-scale shell-model calculations using different sets of two-body matrix elements. In particular, predictions on electromagnetic decay properties such as lifetimes, branching ratios, and mixing ratios are studied in detail.

  9. {alpha} decay of high-spin isomers in superheavy nuclei

    SciTech Connect

    Delion, D. S.; Liotta, R. J.; Wyss, R.

    2007-10-15

    Hindrance factors corresponding to {alpha} decay from two quasiparticle isomeric high K states are evaluated in superheavy nuclei. We found that the hindrance factors are very sensitive to the deformations and, therefore, they may constitute a powerful tool to extract spectroscopic information in these nuclei. The hindrance factors turn out to be very large, specially for nonaligned configurations. This indicates that if one of such states is reached the parent nucleus may become isomeric. It is also possible that {alpha} decay may not proceed through ground state to ground state chains but rather through excited states.

  10. High-spin states in /sup 201,203/At and the systematic behavior of Z = 85 isotopes

    SciTech Connect

    Dybdal, K.; Chapuran, T.; Fossan, D.B.; Piel, W.F. Jr.; Horn, D.; Warburton, E.K.

    1983-09-01

    A spectroscopic investigation of high-spin states in /sup 201,203/At was performed by means of the reactions /sup 192,194/Pt(/sup 14/N,5n)/sup 201,203/At with /sup 14/N energies between 85 and 100 MeV. In-beam measurements of ..gamma..-ray excitation functions, ..gamma..-..gamma.. coincidences, ..gamma..-ray angular distributions, and pulsed-beam-..gamma.. timing were made to determine the decay scheme, level energies, ..gamma..-ray multipolarities, spin-parity assignments, and isomeric lifetimes. The yrast and near-yrast level structures were established up to Japprox.(25/2), and several isomers with mean lifetimes around 20 ns were observed. The systematic trends of level energies of the odd-mass astatine (Z = 85) isotopes are discussed in terms of proton-particle configurations of /sup 211//sub 85/At/sub 126/ coupled to neutron-hole configurations of the corresponding even-mass lead isotones.

  11. PARTICLE-HOLE NATURE OF THE LIGHT HIGH-SPIN TOROIDAL ISOMERS

    SciTech Connect

    Staszczak, A.; Wong, Cheuk-Yin

    2015-01-01

    Nuclei under non-collective rotation with a large angular momentum above some threshold can assume a toroidal shape. In our previous work, we showed by using cranked Skyrme Hartree Fock approach that even even, N = Z, high-K, toroidal isomeric states may have general occurrences for light nuclei with 28 < A < 52. We present here some additional results and systematics on the particle-hole nature of these high-spin toroidal isomers.

  12. A new Skyrme energy density functional for a better description of spin-isospin resonances

    NASA Astrophysics Data System (ADS)

    Roca-Maza, X.; Colò, G.; Cao, Li-Gang; Sagawa, H.

    2015-10-01

    A correct determination of the isospin and spin-isospin properties of the nuclear effective interaction should lead to an accurate description of the Gamow-Teller resonance (GT), the Spin Dipole Resonance (SDR), the Giant Dipole Resonance (GDR) or the Antianalog Giant Dipole Resonance (AGDR), among others. A new Skyrme energy density functional named SAMi is introduced with the aim of going a step forward in setting the bases for a more precise description of spin-isospin resonances [1, 2]. In addition, we will discuss some new features of our analysis on the AGDR in 208Pb [3] as compared with available experimental data on this resonance [4, 5, 6], and on the GDR [7]. Such study, guided by a simple yet physical pocket formula, has been developed by employing the so called SAMi-J family of systematically varied interactions. This set of interactions is compatible with experimental data for values of the symmetry energy at saturation J and slope parameter L falling in the ranges 31-33 MeV and 75-95 MeV, respectively.

  13. A new Skyrme energy density functional for a better description of spin-isospin resonances

    SciTech Connect

    Roca-Maza, X.; Colò, G.; Cao, Li-Gang; Sagawa, H.

    2015-10-15

    A correct determination of the isospin and spin-isospin properties of the nuclear effective interaction should lead to an accurate description of the Gamow-Teller resonance (GT), the Spin Dipole Resonance (SDR), the Giant Dipole Resonance (GDR) or the Antianalog Giant Dipole Resonance (AGDR), among others. A new Skyrme energy density functional named SAMi is introduced with the aim of going a step forward in setting the bases for a more precise description of spin-isospin resonances [1, 2]. In addition, we will discuss some new features of our analysis on the AGDR in {sup 208}Pb [3] as compared with available experimental data on this resonance [4, 5, 6], and on the GDR [7]. Such study, guided by a simple yet physical pocket formula, has been developed by employing the so called SAMi-J family of systematically varied interactions. This set of interactions is compatible with experimental data for values of the symmetry energy at saturation J and slope parameter L falling in the ranges 31−33 MeV and 75−95 MeV, respectively.

  14. Low-energy paramagnetic spin fluctuations in the weak itinerant ferromagnet MnSi

    NASA Astrophysics Data System (ADS)

    Ishikawa, Y.; Noda, Y.; Fincher, C.; Shirane, G.

    1982-01-01

    Low-energy paramagnetic excitations in the weak itinerant ferromagnet (WIF) MnSi have been studied by neutron scattering. The observed spectrum has a Lorentzian form (ΓΓ2+ω2) and is clearly separated from excitations in the Stoner continuum. The generalized susceptibility, χ(q), has been obtained by integrating the scattering intensity over energy. It is found that χ(q) depends upon the wave vector q as χ(q)-1=κ2(T)+q2 for q<=0.125(2πa) with κ2(T)=κ20(T-Tc). After extrapolating these results to q=0, it is found that χ(q=0) follows the Curie-Weiss law, suggesting that the observed spin fluctuations correspond to the Moriya-Kawabata (MK) spin fluctuations responsible for the Curie-Weiss dependence of the static susceptibility of a WIF. The linewidth Γ is found to be proportional to qχ(q) as predicted by the MK theory, in contrast with the q2χ(q) relation expected in a Heisenberg system. These results provide the first direct experimental evidence for the existence of MK spin fluctuations in a WIF above Tc.

  15. Entanglement of two qubits coupled to an XY spin chain: Role of energy current

    NASA Astrophysics Data System (ADS)

    Liu, Ben-Qiong; Shao, Bin; Zou, Jian

    2009-12-01

    We investigate the entanglement dynamics of a two-qubit system which interacts with a Heisenberg XY spin chain constrained to carry an energy current. We show an explicit connection between the decoherence factor and entanglement, and numerically and analytically study the dynamical process of entanglement in both weak- and strong-coupling cases for two initial states, the general pure state and the mixed Werner state. We provide results that the entanglement evolution depends not only on the energy current, the anisotropy parameter and the system-environment couplings but also on the size of degrees of freedom of environment. In particular, our results imply that entanglement will be strongly suppressed by the introduction of energy current on the environmental spin chain in the weak-coupling region while it is not sensitive to the energy current in the strong-coupling region. We also observe the sudden death of entanglement in the system and show how the energy current affects the phenomenon.

  16. Entanglement of two qubits coupled to an XY spin chain: Role of energy current

    SciTech Connect

    Liu Benqiong; Shao Bin; Zou Jian

    2009-12-15

    We investigate the entanglement dynamics of a two-qubit system which interacts with a Heisenberg XY spin chain constrained to carry an energy current. We show an explicit connection between the decoherence factor and entanglement, and numerically and analytically study the dynamical process of entanglement in both weak- and strong-coupling cases for two initial states, the general pure state and the mixed Werner state. We provide results that the entanglement evolution depends not only on the energy current, the anisotropy parameter and the system-environment couplings but also on the size of degrees of freedom of environment. In particular, our results imply that entanglement will be strongly suppressed by the introduction of energy current on the environmental spin chain in the weak-coupling region while it is not sensitive to the energy current in the strong-coupling region. We also observe the sudden death of entanglement in the system and show how the energy current affects the phenomenon.

  17. High energy polarized beams from hyperon decays

    SciTech Connect

    Underwood, D.G.

    1986-01-01

    The use of various ways to utilize lambda decays to obtain polarized beams of protons and antiprotons is emphasized. Examples described are the Fermilab polarized beam, now under construction, and the use of similar techniques at other energies. Beam transport, spin precession and reversal systems, and polarimeters are also discussed. 8 refs., 4 figs.

  18. Nutation and precession control of the High Energy Solar Physics (HESP) satellite

    NASA Technical Reports Server (NTRS)

    Jayaraman, C. P.; Robertson, B. P.

    1993-01-01

    The High Energy Solar Physics (HESP) spacecraft is an intermediate class satellite proposed by NASA to study solar high-energy phenomena during the next cycle of high solar activity in the 1998 to 2005 time frame. The HESP spacecraft is a spinning satellite which points to the sun with stringent pointing requirements. The natural dynamics of a spinning satellite includes an undesirable effect: nutation, which is due to the presence of disturbances and offsets of the spin axis from the angular momentum vector. The proposed Attitude Control System (ACS) attenuates nutation with reaction wheels. Precessing the spacecraft to track the sun in the north-south and east-west directions is accomplished with the use of torques from magnetic torquer bars. In this paper, the basic dynamics of a spinning spacecraft are derived, control algorithms to meet HESP science requirements are discussed and simulation results to demonstrate feasibility of the ACS concept are presented.

  19. Thermodynamic properties of highly frustrated quantum spin ladders: Influence of many-particle bound states

    NASA Astrophysics Data System (ADS)

    Honecker, A.; Wessel, S.; Kerkdyk, R.; Pruschke, T.; Mila, F.; Normand, B.

    2016-02-01

    Quantum antiferromagnets have proven to be some of the cleanest realizations available for theoretical, numerical, and experimental studies of quantum fluctuation effects. At finite temperatures, however, the additional effects of thermal fluctuations in the restricted phase space of a low-dimensional system have received much less attention, particularly the situation in frustrated quantum magnets, where the excitations may be complex collective (bound or even fractionalized) modes. We investigate this problem by studying the thermodynamic properties of the frustrated two-leg S =1/2 spin ladder, with particular emphasis on the fully frustrated case. We present numerical results for the magnetic specific heat and susceptibility, obtained from exact diagonalization and quantum Monte Carlo studies, which we show can be rendered free of the sign problem even in a strongly frustrated system and which allow us to reach unprecedented sizes of L =200 ladder rungs. We find that frustration effects cause an unconventional evolution of the thermodynamic response across the full parameter regime of the model. However, close to the first-order transition they cause a highly anomalous reduction in temperature scales with no concomitant changes in the gap; the specific heat shows a very narrow peak at very low energies and the susceptibility rises abruptly at extremely low temperatures. Unusually, the two quantities have different gaps over an extended region of the parameter space. We demonstrate that these results reflect the presence of large numbers of multiparticle bound-state excitations, whose energies fall below the one-triplon gap in the transition region.

  20. High spin spectroscopy for A approx 160 nuclei

    SciTech Connect

    Yu, C.-H. Tennessee Univ., Knoxville, TN . Dept. of Physics and Astronomy); Gascon, J.; Garrett, J.D.; Hagemann, G.B. )

    1989-01-01

    Experimental routhians, alignments, band crossing frequencies, and the B(M1)/B(E2) ratios of the N = 90 isotopes and several light Lu (N = 90--96) isotopes are summarized and discussed in terms of shape changes. These systematic analyses show a neutron and proton number dependent deformations (both quadruple and {gamma} deformations) for these light rare earth nuclei. The stability of the nuclear deformation with respect to {beta} and {gamma} is also found to be particle number dependent. Such particle number dependent shapes can be attributed to the different locations of the proton and neutron Fermi levels in the Nilsson diagrams. Configurations dependent shapes are discussed specially concerned the deformation difference between the proton h{sub 9/2}1/2{sup -}(541) and the high-K h{sub 11/2} configurations. The observed large neutron band crossing frequencies in the h{sub 9/2}1/2{sup -}(541) configuration support the predicted large deformation of this configuration but can be reproduced by the cranked shell model calculation according to the predicted deformations. Lifetime measurement for {sup 157}Ho, one of the nuclei that show a large {h bar}{omega}{sup c} in the 1/2{sup -}(541) band, indicates that deformation difference can only account for 20% of such shift in {h bar}{omega}{sub c}. 55 refs., 12 figs.

  1. High energy high brightness thin disk laser

    NASA Astrophysics Data System (ADS)

    Nixon, Matthew D.; Cates, Michael C.

    2012-11-01

    Boeing has been developing solid state lasers for high energy applications since 2004 using Yb:YAG thin disk lasers as pioneered by A. Giesen1 and commercialized by Trumpf Laser GmbH.2 In this paper, we report results of our second generation design and status of a third generation we are currently developing, which will produce 35 kW and a beam quality <2.

  2. Widespread spin polarization effects in photoemission from topological insulators

    SciTech Connect

    Jozwiak, C.; Chen, Y. L.; Fedorov, A. V.; Analytis, J. G.; Rotundu, C. R.; Schmid, A. K.; Denlinger, J. D.; Chuang, Y.-D.; Lee, D.-H.; Fisher, I. R.; Birgeneau, R. J.; Shen, Z.-X.; Hussain, Z.; Lanzara, A.

    2011-06-22

    High-resolution spin- and angle-resolved photoemission spectroscopy (spin-ARPES) was performed on the three-dimensional topological insulator Bi{sub 2}Se{sub 3} using a recently developed high-efficiency spectrometer. The topological surface state's helical spin structure is observed, in agreement with theoretical prediction. Spin textures of both chiralities, at energies above and below the Dirac point, are observed, and the spin structure is found to persist at room temperature. The measurements reveal additional unexpected spin polarization effects, which also originate from the spin-orbit interaction, but are well differentiated from topological physics by contrasting momentum and photon energy and polarization dependencies. These observations demonstrate significant deviations of photoelectron and quasiparticle spin polarizations. Our findings illustrate the inherent complexity of spin-resolved ARPES and demonstrate key considerations for interpreting experimental results.

  3. Laser induced spin precession in highly anisotropic granular L1{sub 0} FePt

    SciTech Connect

    Becker, J.; Mosendz, O.; Weller, D.; Kirilyuk, A.; Rasing, Th.; Kimel, A.; Maan, J. C.; Christianen, P. C. M.

    2014-04-14

    The dynamic magnetic properties of a highly anisotropic, granular L1{sub 0} FePt thin film in magnetic fields up to 7 T are investigated using time-resolved magneto-optical Kerr effect measurements. We find that ultrashort laser pulses induce coherent spin precession in the granular FePt sample. Frequencies of spin precession up to over 400 GHz are observed, which are strongly field and temperature dependent. The high frequencies can be ascribed to the high value of the magnetocrystalline anisotropy constant K{sub u} leading to large anisotropy fields H{sub a} of up to 10.7 T at 170 K. A Gilbert damping parameter of α ∼ 0.1 was derived from the lifetimes of the oscillations.

  4. Novel multipole Wien filter as three-dimensional spin manipulator

    SciTech Connect

    Yasue, T. Suzuki, M.; Koshikawa, T.; Tsuno, K.; Goto, S.; Arai, Y.

    2014-04-15

    Spin polarized electron beam is often used in material characterizations which relates to magnetism as well as in the high energy particle physics. The manipulation of the spin polarization toward the arbitrary direction is indispensable in such studies. In the present work, a novel multipole Wien filter is proposed as the three-dimensional spin manipulator, and a prototype 8-pole Wien filter is developed. It is applied to spin polarized low energy electron microscopy, and the variation of the magnetic contrast with managing the spin polarization is evaluated. It is confirmed that the novel multipole Wien filter can manipulate the spin polarization three-dimensionally.

  5. Equation of State and Spin Transition of (Mg,Fe)O at High Pressures

    NASA Astrophysics Data System (ADS)

    Solomatova, N. V.; Jackson, J. M.; Sturhahn, W.; Zhao, J.; Toellner, T.; Kalkan, B.; Wicks, J. K.; Steinhardt, W.

    2014-12-01

    Earth's lower mantle occupies more than half of Earth's volume, and is composed primarily of bridgmanites and (Mg,Fe)O "ferropericlase." Knowledge of the behavior of lower mantle minerals is essential for interpreting complexity in the deep Earth. Although it is suggested that (Mg,Fe)O represents a major volume fraction of Earth's interior, the iron concentration of (Mg,Fe)O is not very well constrained at all depths of the lower mantle. Near the base of the lower mantle, an enhanced iron content may be found due to melting events in Earth's history and/or reactions with the iron-dominant liquid outer core. Here we examine the high-pressure behavior of polycrystalline (Mg,Fe)O containing 48 mol% FeO ("FP48"), loaded hydrostatically with neon as a pressure medium. Using x-ray diffraction and synchrotron Mössbauer spectroscopy we measure the equation of state of FP48 to about 80 GPa at 300 K and hyperfine parameters to 100 GPa at 300 K, respectively. A gradual volume drop is observed between ˜55 and 75 GPa. To confirm that the observed volume drop is due to a spin crossover, the quadrupole splitting (QS) and isomer shift (IS) of Fe2+ are determined as a function of pressure. At low pressures, our spectra are fitted with two Fe2+-like sites. At pressures between 43 and 81 GPa, an additional Fe2+-like site with a QS of 0 is required, indicative of low-spin iron. Above 93 GPa, two low-spin Fe2+-like sites explain the data well, signifying the completion of the spin crossover. Using a spin crossover equation of state, we have determined the volume drop at the calculated transition pressure and the relevant elastic properties of FP48. Our results are compared to previous measurements of (Mg,Fe)O with varying concentrations of iron at high pressures.

  6. ^129Xe-Rb spin-exchange cross section measurement at high magnetic field

    NASA Astrophysics Data System (ADS)

    Jau, Yuan-Yu; Kuzma, N. N.; Walter, D. K.; Griffith, W. M.; Happer, W.

    2002-05-01

    We report NMR measurements of the velocity-averaged ^129Xe-Rb spin-exchange cross section <σ_exv> using isotopically enriched xenon gas in a sealed aluminosilicate cell. At 9.4 T, it is possible to detect Boltzmann polarization of xenon gas nuclei without optical pumping. Over the temperature range from 160 to 200^rcC, binary collisions with Rb atoms dominate the ^129Xe spin-relaxation rate (1/T_1) through spin-exchange. Our data show that the spin-exchange contribution of van der Waals RbXe molecules at high magnetic field is very small compared to the contribition of binary collisions. From the observed linear dependence of 1/T1 on Rb density, we extract the value <σ_exv>=1.720.29× 10-16 cm^3/sec at 180^rcC and 9.4 T, where we deduce the Rb number density from our Faraday rotation measurements. In addition, we discuss a theoretical prediction of <σ_exv> based on our numerical computations and compare it to the experimental result.

  7. Revisiting spin-lattice relaxation time measurements for dilute spins in high-resolution solid-state NMR spectroscopy

    NASA Astrophysics Data System (ADS)

    Fu, Riqiang; Li, Jun; Cui, Jingyu; Peng, Xinhua

    2016-07-01

    Numerous nuclear magnetic resonance (NMR) measurements of spin-lattice relaxation times (T1S) for dilute spins such as 13C have led to investigations of the motional dynamics of individual functional groups in solid materials. In this work, we revisit the Solomon equations and analyze how the heteronuclear cross relaxation between the dilute S (e.g. 13C) and abundant I (e.g. 1H) spins affects the measured T1S values in solid-state NMR in the absence of 1H saturation during the recovery time. It is found theoretically that at the beginning of the S spin magnetization recovery, the existence of non-equilibrium I magnetization introduces the heteronuclear cross relaxation effect onto the recovery of the S spin magnetization and confirmed experimentally that such a heteronuclear cross relaxation effect results in the recovery overshoot phenomena for the dilute spins when T1S is on the same order of T1H, leading to inaccurate measurements of the T1S values. Even when T1S is ten times larger than T1H, the heteronuclear cross relaxation effect on the measured T1S values is still noticeable. Furthermore, this cross relaxation effect on recovery trajectory of the S spins can be manipulated and even suppressed by preparing the initial I and S magnetization, so as to obtain the accurate T1S values. A sample of natural abundance L-isoleucine powder has been used to demonstrate the T1S measurements and their corresponding measured T1C values under various experimental conditions.

  8. Revisiting spin-lattice relaxation time measurements for dilute spins in high-resolution solid-state NMR spectroscopy.

    PubMed

    Fu, Riqiang; Li, Jun; Cui, Jingyu; Peng, Xinhua

    2016-07-01

    Numerous nuclear magnetic resonance (NMR) measurements of spin-lattice relaxation times (T1S) for dilute spins such as (13)C have led to investigations of the motional dynamics of individual functional groups in solid materials. In this work, we revisit the Solomon equations and analyze how the heteronuclear cross relaxation between the dilute S (e.g. (13)C) and abundant I (e.g. (1)H) spins affects the measured T1S values in solid-state NMR in the absence of (1)H saturation during the recovery time. It is found theoretically that at the beginning of the S spin magnetization recovery, the existence of non-equilibrium I magnetization introduces the heteronuclear cross relaxation effect onto the recovery of the S spin magnetization and confirmed experimentally that such a heteronuclear cross relaxation effect results in the recovery overshoot phenomena for the dilute spins when T1S is on the same order of T1H, leading to inaccurate measurements of the T1S values. Even when T1S is ten times larger than T1H, the heteronuclear cross relaxation effect on the measured T1S values is still noticeable. Furthermore, this cross relaxation effect on recovery trajectory of the S spins can be manipulated and even suppressed by preparing the initial I and S magnetization, so as to obtain the accurate T1S values. A sample of natural abundance l-isoleucine powder has been used to demonstrate the T1S measurements and their corresponding measured T1C values under various experimental conditions. PMID:27187211

  9. Magic radio-frequency dressing of nuclear spins in high-accuracy optical clocks.

    PubMed

    Zanon-Willette, Thomas; de Clercq, Emeric; Arimondo, Ennio

    2012-11-30

    A Zeeman-insensitive optical clock atomic transition is engineered when nuclear spins are dressed by a nonresonant radio-frequency field. For fermionic species as (87)Sr, (171)Yb, and (199)Hg, particular ratios between the radio-frequency driving amplitude and frequency lead to "magic" magnetic values where a net cancelation of the Zeeman clock shift and a complete reduction of first-order magnetic variations are produced within a relative uncertainty below the 10(-18) level. An Autler-Townes continued fraction describing a semiclassical radio-frequency dressed spin is numerically computed and compared to an analytical quantum description including higher-order magnetic field corrections to the dressed energies. PMID:23368116

  10. Transition from collective to noncollective rotation at high spin in N approx. = 87 nuclei

    SciTech Connect

    Baktash, C.

    1982-01-01

    The systematics of the (E2) ..gamma.. ray transition energies and the available lifetime data are used to characterize the excitation modes of the light rare-earth nuclei (N greater than or equal to 82) at different spins. The results, which include our recently obtained data on /sup 149/Gd, /sup 154/Ho, /sup 155/Er, /sup 157/Yb and /sup 158/Yb nuclei, indicate that, at low spins, the nuclear excitation mode (shapes) change from single-particle excitations (weakly oblate) in N less than or equal to 85 nuclei to quasi-vibrational (soft triaxial) in N = 86, weakly rotational (prolate) in N = 87, and rotational (prolate) in the N greater than or equal to 88 systems. At higher angular momenta, all these nuclei show a general tendency to traverse the (epsilon,..gamma..) plane towards the oblate axis, and to eventually adopt the aligned coupling mode of excitation.

  11. Quasiparticle band gap of organic-inorganic hybrid perovskites: Crystal structure, spin-orbit coupling, and self-energy effects

    NASA Astrophysics Data System (ADS)

    Gao, Weiwei; Gao, Xiang; Abtew, Tesfaye; Sun, Yiyang; Zhang, Shengbai; Zhang, Peihong

    The quasiparticle band gaps of organic-inorganic hybrid perovskites are often determined (and can be controlled) by various factors, complicating predictive materials optimization. Here we report a comprehensive investigation on the band gap formation mechanism in CH3NH3PbI3 by decoupling various contributing factors which ultimately determine their electronic structure and quasiparticle band gap. Four major factors, namely, quasiparticle self-energy, spin-orbit coupling, volume (lattice constant) effects, and structural distortions due to the presence of organic molecules, and their influences on the quasiparticle band structure of organometal hybrid perovskites are illustrated. We find that although methylammonium cations do not contribute directly to the electronic states near band edges, they play an important role in defining the band gap through a lattice distortion mechanism and by controlling the overall lattice constants (thus the chemical bonding of the optically active PbI3-). The spin-orbit coupling effects drastically reduce the electron and hole effective masses in these systems, which is beneficial for high carrier mobilities and small exciton binding energies. This work is supported by the National Natural Science Foundation of China (Grant No. 11328401), NSF (Grant No. DMR-0946404 and DMR-1506669), and the SUNY Networks of Excellence.

  12. High flux solar energy transformation

    DOEpatents

    Winston, Roland; Gleckman, Philip L.; O'Gallagher, Joseph J.

    1991-04-09

    Disclosed are multi-stage systems for high flux transformation of solar energy allowing for uniform solar intensification by a factor of 60,000 suns or more. Preferred systems employ a focusing mirror as a primary concentrative device and a non-imaging concentrator as a secondary concentrative device with concentrative capacities of primary and secondary stages selected to provide for net solar flux intensification of greater than 2000 over 95 percent of the concentration area. Systems of the invention are readily applied as energy sources for laser pumping and in other photothermal energy utilization processes.

  13. High flux solar energy transformation

    DOEpatents

    Winston, R.; Gleckman, P.L.; O'Gallagher, J.J.

    1991-04-09

    Disclosed are multi-stage systems for high flux transformation of solar energy allowing for uniform solar intensification by a factor of 60,000 suns or more. Preferred systems employ a focusing mirror as a primary concentrative device and a non-imaging concentrator as a secondary concentrative device with concentrative capacities of primary and secondary stages selected to provide for net solar flux intensification of greater than 2000 over 95 percent of the concentration area. Systems of the invention are readily applied as energy sources for laser pumping and in other photothermal energy utilization processes. 7 figures.

  14. Extraterrestrial high energy neutrino fluxes

    NASA Technical Reports Server (NTRS)

    Stecker, F. W.

    1979-01-01

    Using the most recent cosmic ray spectra up to 2x10 to the 20th power eV, production spectra of high energy neutrinos from cosmic ray interactions with interstellar gas and extragalactic interactions of ultrahigh energy cosmic rays with 3K universal background photons are presented and discussed. Estimates of the fluxes from cosmic diffuse sources and the nearby quasar 3C273 are made using the generic relationship between secondary neutrinos and gammas and using recent gamma ray satellite data. These gamma ray data provide important upper limits on cosmological neutrinos. Quantitative estimates of the observability of high energy neutrinos from the inner galaxy and 3C273 above atmospheric background for a DUMAND type detector are discussed in the context of the Weinberg-Salam model with sq sin theta omega = 0.2 and including the atmospheric background from the decay of charmed mesons. Constraints on cosmological high energy neutrino production models are also discussed. It appears that important high energy neutrino astronomy may be possible with DUMAND, but very long observing times are required.

  15. Overview of spin physics

    SciTech Connect

    Yokosawa, A.

    1992-12-23

    Spin physics activities at medium and high energies became significantly active when polarized targets and polarized beams became accessible for hadron-hadron scattering experiments. My overview of spin physics will be inclined to the study of strong interaction using facilities at Argonne ZGS, Brookhaven AGS (including RHIC), CERN, Fermilab, LAMPF, an SATURNE. In 1960 accelerator physicists had already been convinced that the ZGS could be unique in accelerating a polarized beam; polarized beams were being accelerated through linear accelerators elsewhere at that time. However, there was much concern about going ahead with the construction of a polarized beam because (i) the source intensity was not high enough to accelerate in the accelerator, (ii) the use of the accelerator would be limited to only polarized-beam physics, that is, proton-proton interaction, and (iii) p-p elastic scattering was not the most popular topic in high-energy physics. In fact, within spin physics, [pi]-nucleon physics looked attractive, since the determination of spin and parity of possible [pi]p resonances attracted much attention. To proceed we needed more data beside total cross sections and elastic differential cross sections; measurements of polarization and other parameters were urgently needed. Polarization measurements had traditionally been performed by analyzing the spin of recoil protons. The drawbacks of this technique are: (i) it involves double scattering, resulting in poor accuracy of the data, and (ii) a carbon analyzer can only be used for a limited region of energy.

  16. High-spin diimine complexes of iron(II) reject binding of carbon monoxide: theoretical analysis of thermodynamic factors inhibiting or favoring spin-crossover.

    PubMed

    Hardman, Ned J; Fang, Xinggao; Scott, Brian L; Wright, Robert J; Martin, Richard L; Kubas, Gregory J

    2005-11-14

    A new series of Fe(II) complexes, FeCl2[N(R)=C(Me)C(Me)=N(R)], containing diimine ligands with hemilabile sidearms R (R = CH2(CH2)2NMe2, 1, CH2(CH2)2OMe, 2, CH2(CH2)2SMe), 3) were synthesized. The crystal structure of 1 showed 6-coordination where both amine arms were attached, whereas 2 was a 5-coordinate 16e species with one methoxy arm dangling free. Extensive attempts were made to bind CO to these species to synthesize precursors for dihydrogen complexes but were unsuccessful. Reaction of 1 with 1 or 2 equiv of AgOTf under CO atmosphere resulted in isolation of only a 6-coordinate bis(triflate)-containing product [Fe[N(R)=C(Me)C(Me)=N(R)](OTf)2] (R = CH2(CH2)2NMe2), 5. Reaction of 5-coordinate 2 with AgSbF6 under CO did not give a CO adduct but afforded instead a dicationic dinuclear complex [Fe[N(R)=C(Me)C(Me)=N(R)](mu-Cl)]2[SbF6]2 (R = CH2(CH2)2OMe), 4, containing a weakly bound SbF6. Thus coordination of hard-donor anions to iron was favored over CO binding. The unexpected rejection of binding of CO is rationalized by the iron being in a high-spin state in this system and energetically incapable of spin crossover to a low-spin state. Theoretical calculations on CO interaction with Fe(II) centers in spin states S = 0, 1, and 2 for both the 16e complexes and their CO adducts aid further understanding of this problem. They show that interaction of CO with a high-spin 5-coordinate Fe model diimine complex is essentially thermoneutral but is exergonic by about 48 kcal/mol to a comparable but low-spin diphosphine fragment. Spin crossover is thus disfavored thermodynamically rather than kinetically (e.g. a "spin block" effect); i.e., the ligand field strengths of the primarily N-donor groups are apparently insufficient to give a low-spin CO adduct. PMID:16270969

  17. High Energy Astrophysics Program (HEAP)

    NASA Technical Reports Server (NTRS)

    Angelini, Lorella; Corcoran, Michael; Drake, Stephen; McGlynn, Thomas A.; Snowden, Stephen; Mukai, Koji; Cannizzo, John; Lochner, James; Rots, Arnold; Christian, Eric; Barthelmy, Scott; Palmer, David; Mitchell, John; Esposito, Joseph; Sreekumar, P.; Hua, Xin-Min; Mandzhavidze, Natalie; Chan, Kai-Wing; Soong, Yang; Barrett, Paul

    1998-01-01

    This report reviews activities performed by the members of the USRA contract team during the 6 months of the reporting period and projected activities during the coming 6 months. Activities take place at the Goddard Space Flight Center, within the Laboratory for High Energy Astrophysics. Developments concern instrumentation, observation, data analysis, and theoretical work in astrophysics. Supported missions include advanced Satellite for Cosmology and Astrophysics (ASCA), X-Ray Timing Experiment (XTE), X-Ray Spectrometer (XRS), Astro-E, High Energy Astrophysics Science Archive Research Center (HEASARC) and others.

  18. High Energy Astrophysics Program (HEAP)

    NASA Technical Reports Server (NTRS)

    Angelini, L.; Holdridge, David V.; Norris, J. (Technical Monitor)

    1998-01-01

    This report reviews activities performed by members of the USRA contract team during the six months of the reporting period and projected activities during the coming six months. Activities take place at the Goddard Space Flight Center, within the Laboratory for High Energy Astrophysics. Developments concern instrumentation, observation, data analysis, and theoretical work in Astrophysics Missions supported include: Advanced Satellite for Cosmology and Astrophysics (ASCA), X-ray Timing Experiment (XTE), X-ray Spectrometer (XRS), Astro-E, High Energy Astrophysics Science Archive Research Center (HEASARC), and others.

  19. Stanene cyanide: a novel candidate of Quantum Spin Hall insulator at high temperature.

    PubMed

    Ji, Wei-Xiao; Zhang, Chang-Wen; Ding, Meng; Li, Ping; Li, Feng; Ren, Miao-Juan; Wang, Pei-Ji; Hu, Shu-Jun; Yan, Shi-Shen

    2015-01-01

    The search for quantum spin Hall (QSH) insulators with high stability, large and tunable gap and topological robustness, is critical for their realistic application at high temperature. Using first-principle calculations, we predict the cyanogen saturated stanene SnCN as novel topological insulators material, with a bulk gap as large as 203 meV, which can be engineered by applying biaxial strain and electric field. The band topology is identified by Z2 topological invariant together with helical edge states, and the mechanism is s-pxy band inversion at G point induced by spin-orbit coupling (SOC). Remarkably, these systems have robust topology against chemical impurities, based on the calculations on halogen and cyano group co-decorated stanene SnXxX'1-x (X,X'  =  F, Cl, Br, I and CN), which makes it an appropriate and flexible candidate material for spintronic devices. PMID:26688269

  20. High-spin γ-ray spectroscopy in the vicinity of 56Ni

    NASA Astrophysics Data System (ADS)

    Rudolph, D.; Baktash, C.; Satuła, W.; Dobaczewski, J.; Nazarewicz, W.; Brinkman, M. J.; Devlin, M.; Jin, H.-Q.; LaFosse, D. R.; Riedinger, L. L.; Sarantites, D. G.; Yu, C.-H.

    1998-02-01

    High-spin states of a number of nuclei near 56Ni have been studied by means of the 28Si( 36Ar,x αypzn) reaction. The GAMMASPHERE array in conjunction with light charged-particle and neutron detectors were used to identify and cleanly select the fusion-evaporation products. In addition to significantly extending the level schemes of many previously known N = Z nuclei from 52Fe to 58Cu, excited states in the one-neutron-hole nucleus 55Ni and high-spin rotational bands in the vicinity of the doubly-magic 56Ni have been established for the first time. Spherical- fp shell model and cranked Hartree-Fock calculations employing several Skyrme-type effective interactions have been used to interpret these data. The calculated moments of inertia of the rotational bands show considerable sensitivity to the details of the effective interactions.

  1. Levels in 210Fr and the decay of a high-spin, multi-particle isomer

    NASA Astrophysics Data System (ADS)

    Margerin, V.; Lane, G. J.; Dracoulis, G. D.; Palalani, N.; Smith, M. L.

    2012-10-01

    The structure of 210Fr has been studied through the 197Au(18O, 5n)210Fr reaction. A high-spin isomeric state has been identified at ~4.4 MeV. It has a lifetime of 686(17) ns and decays by two γ-rays that are very likely to be either M2 or E3 multipolarity. The measured strengths in the case of E3 assignments are approximatively 8 and 21 W.u., respectively. These would be less enhanced than is observed in the decay from the high spin isomers in 209Fr and 211Fr that are believed to be from a related configuration. Possible configuration assignments are discussed.

  2. Large Magnetoresistance at High Bias Voltage in Double-layer Organic Spin Valves

    NASA Astrophysics Data System (ADS)

    Subedi, R. C.; Liang, S. H.; Geng, R.; Zhang, Q. T.; Lou, L.; Wang, J.; Han, X. F.; Nguyen, T. D.

    We report studies of magnetoresistance (MR) in double-layer organic spin valves (DOSV) using tris (8-hydroxyquinolinato) aluminum (Alq3) spacers. The device exhibits three distinct resistance levels depending on the relative magnetizations of the ferromagnetic electrodes. We observed a much weaker bias voltage dependence of MR in the device compared to that in the conventional organic spin valve (OSV). The MR magnitude reduces by the factor of two at 0.7 V bias voltage in the DOSV compared to 0.02 V in the conventional OSV. Remarkably, the MR magnitude reaches 0.3% at 6 V bias in the DOSVs, the largest MR response ever reported in OSVs at this bias. Our finding may have a significant impact on achieving high efficient bipolar OSVs strictly performed at high voltages. University of Georgia start-up fund, Ministry of Education, Singapore, National Natural Science Foundation of China.

  3. High-performance spinning device for DVD-based micromechanical signal transduction

    NASA Astrophysics Data System (ADS)

    Hwu, En-Te; Chen, Ching-Hsiu; Bosco, Filippo G.; Wang, Wei-Min; Ko, Hsien-Chen; Hwang, Ing-Shouh; Boisen, Anja; Huang, Kuang-Yuh

    2013-04-01

    Here we report a high-throughput spinning device for nanometric scale measurements of microstructures with instrumentation details and experimental results. The readout technology implemented in the designed disc-like device is based on a DVD data storage optical pick-up unit (OPU). With a spinning mechanism, this device can simultaneously measure surface topography, mechanical deflections and resonance frequencies of several microfabricated beams at a high speed. In biochemical sensing applications, the OPU can measure bending changes of functionalized microcantilevers, providing a statistically robust and label-free bio-detection analysis of multiple compounds. The signal-to-noise ratio (S/N) is demonstrated from statistical measurements as 1.2 with arginine detection at 750 nM concentration. Practically, the OPU can measure up to 480 individual cantilever sensors per second with nanometer resolution. The opto-mechanical optimization of the device design and settings for biochemical detection are described.

  4. Stanene cyanide: a novel candidate of Quantum Spin Hall insulator at high temperature

    NASA Astrophysics Data System (ADS)

    Ji, Wei-Xiao; Zhang, Chang-Wen; Ding, Meng; Li, Ping; Li, Feng; Ren, Miao-Juan; Wang, Pei-Ji; Hu, Shu-Jun; Yan, Shi-Shen

    2015-12-01

    The search for quantum spin Hall (QSH) insulators with high stability, large and tunable gap and topological robustness, is critical for their realistic application at high temperature. Using first-principle calculations, we predict the cyanogen saturated stanene SnCN as novel topological insulators material, with a bulk gap as large as 203 meV, which can be engineered by applying biaxial strain and electric field. The band topology is identified by Z2 topological invariant together with helical edge states, and the mechanism is s-pxy band inversion at G point induced by spin-orbit coupling (SOC). Remarkably, these systems have robust topology against chemical impurities, based on the calculations on halogen and cyano group co-decorated stanene SnXxX‧1-x (X,X‧  =  F, Cl, Br, I and CN), which makes it an appropriate and flexible candidate material for spintronic devices.

  5. Stanene cyanide: a novel candidate of Quantum Spin Hall insulator at high temperature

    PubMed Central

    Ji, Wei-xiao; Zhang, Chang-wen; Ding, Meng; Li, Ping; Li, Feng; Ren, Miao-juan; Wang, Pei-ji; Hu, Shu-jun; Yan, Shi-shen

    2015-01-01

    The search for quantum spin Hall (QSH) insulators with high stability, large and tunable gap and topological robustness, is critical for their realistic application at high temperature. Using first-principle calculations, we predict the cyanogen saturated stanene SnCN as novel topological insulators material, with a bulk gap as large as 203 meV, which can be engineered by applying biaxial strain and electric field. The band topology is identified by Z2 topological invariant together with helical edge states, and the mechanism is s-pxy band inversion at G point induced by spin-orbit coupling (SOC). Remarkably, these systems have robust topology against chemical impurities, based on the calculations on halogen and cyano group co-decorated stanene SnXxX′1−x (X,X′  =  F, Cl, Br, I and CN), which makes it an appropriate and flexible candidate material for spintronic devices. PMID:26688269

  6. High-pressure, high-temperature magic angle spinning nuclear magnetic resonance devices and processes for making and using same

    DOEpatents

    Hu, Jian Zhi; Hu, Mary Y.; Townsend, Mark R.; Lercher, Johannes A.; Peden, Charles H. F.

    2015-10-06

    Re-usable ceramic magic angle spinning (MAS) NMR rotors constructed of high-mechanic strength ceramics are detailed that include a sample compartment that maintains high pressures up to at least about 200 atmospheres (atm) and high temperatures up to about least about 300.degree. C. during operation. The rotor designs minimize pressure losses stemming from penetration over an extended period of time. The present invention makes possible a variety of in-situ high pressure, high temperature MAS NMR experiments not previously achieved in the prior art.

  7. Dynamics of Bound Monopoles in Artificial Spin Ice: How to Store Energy in Dirac Strings

    NASA Astrophysics Data System (ADS)

    Vedmedenko, E. Y.

    2016-02-01

    Dirac strings in spin ices are lines of reversed dipoles joining two quasiparticle excitations. These excitations behave as unbound emergent monopoles if the tension of Dirac strings vanishes. In this Letter, analytical and numerical analysis are used to study the dynamics of two-dimensional dipolar spin ices, artificially created analogs of bulk spin ice, in the regime of bound monopoles. It is shown that, in this regime, strings, rather than monopoles, are effective degrees of freedom explaining the finite-width band of Pauling states. A measurable prediction of path-time dependence of endpoints of a stretched and, then, released Dirac string is made and verified via simulations. It is shown that string dynamics is defined by the characteristic tension-to-mass ratio, which is determined by the fine structure constant and lattice dependent parameter. It is proposed to use string tension to achieve spontaneous magnetic currents. A concept of an energy storing device on the basis of this principle is proposed and illustrated by an experimental demonstration. A scheme of independent measurement at the nanoscale is proposed.

  8. Dynamics of Bound Monopoles in Artificial Spin Ice: How to Store Energy in Dirac Strings.

    PubMed

    Vedmedenko, E Y

    2016-02-19

    Dirac strings in spin ices are lines of reversed dipoles joining two quasiparticle excitations. These excitations behave as unbound emergent monopoles if the tension of Dirac strings vanishes. In this Letter, analytical and numerical analysis are used to study the dynamics of two-dimensional dipolar spin ices, artificially created analogs of bulk spin ice, in the regime of bound monopoles. It is shown that, in this regime, strings, rather than monopoles, are effective degrees of freedom explaining the finite-width band of Pauling states. A measurable prediction of path-time dependence of endpoints of a stretched and, then, released Dirac string is made and verified via simulations. It is shown that string dynamics is defined by the characteristic tension-to-mass ratio, which is determined by the fine structure constant and lattice dependent parameter. It is proposed to use string tension to achieve spontaneous magnetic currents. A concept of an energy storing device on the basis of this principle is proposed and illustrated by an experimental demonstration. A scheme of independent measurement at the nanoscale is proposed. PMID:26943555

  9. High power ferromagnetic resonance and spin wave instability processes in Permalloy thin films

    NASA Astrophysics Data System (ADS)

    An, Sung Yong; Krivosik, Pavol; Kraemer, Michael A.; Olson, Heidi M.; Nazarov, Alexey V.; Patton, Carl E.

    2004-08-01

    The high power ferromagnetic resonance (FMR) response, as well as butterfly curves of the spin wave instability threshold microwave field amplitude hcrit versus in-plane static field H profiles, have been measured for Permalloy films with thicknesses of 104, 128, and 270nm at a nominal pumping frequency of 9.37GHz. The hcrit values range from about 1 to 7Oe. Both the resonance saturation response at the FMR field and the subsidiary absorption (SA) response for static fields below the FMR field are similar in appearance to those for bulk ferrites. Butterfly curves over the SA response region, while similar to those for ferrites, exhibit a film thickness dependent band edge cutoff effect not found in bulk ferrites. The SA butterfly curve data were analyzed on the basis of a spin wave instability theory adapted to thin films. The observed shift in the SA band edge cutoff with thickness agrees with calculations based on the thin film dispersion response and the assumption of first order instability processes with critical modes at one half the pumping frequency. The fitted SA spin wave linewidths give values consistent with metallic relaxation processes, but indicate critical modes with wave vectors that always make relatively small 0°-20° angles with the static field, very different from the critical modes for bulk ferrites. Three key conclusions from this work are (1) the nonlinear microwave FMR response in Permalloy films is a threshold effect related to well established spin wave instability processes, (2) the details of the SA response are controlled largely by the thin film spin wave dispersion, and (3) these nonlinear processes occur for very small precession angles.

  10. Perfect spin filtering controlled by an electric field in a bilayer graphene junction: Effect of layer-dependent exchange energy

    NASA Astrophysics Data System (ADS)

    Kitakorn, Jatiyanon; I-Ming, Tang; Bumned, Soodchomshom

    2016-07-01

    Magneto transport of carriers with a spin-dependent gap in a ferromagnetic-gated bilayer of graphene is investigated. We focus on the effect of an energy gap induced by the mismatch of the exchange fields in the top and bottom layers of an AB-stacked graphene bilayer. The interplay of the electric and exchange fields causes the electron to acquire a spin-dependent energy gap. We find that, only in the case of the anti-parallel configuration, the effect of a magnetic-induced gap will give rise to perfect spin filtering controlled by the electric field. The resolution of the spin filter may be enhanced by varying the bias voltage. Perfect switching of the spin polarization from + 100% to ‑100% by reversing the direction of electric field is predicted. Giant magnetoresistance is predicted to be easily realized when the applied electric field is smaller than the magnetic energy gap. It should be pointed out that the perfect spin filter is due to the layer-dependent exchange energy. This work points to the potential application of bilayer graphene in spintronics. Project supported by the Kasetsart University Research and Development Institute (KURDI) and Thailand Research Fund (TRF) (Grant No. TRG5780274).

  11. NMR high-resolution magic angle spinning rotor design for quantification of metabolic concentrations

    NASA Astrophysics Data System (ADS)

    Holly, R.; Damyanovich, A.; Peemoeller, H.

    2006-05-01

    A new high-resolution magic angle spinning nuclear magnetic resonance technique is presented to obtain absolute metabolite concentrations of solutions. The magnetic resonance spectrum of the sample under investigation and an internal reference are acquired simultaneously, ensuring both spectra are obtained under the same experimental conditions. The robustness of the technique is demonstrated using a solution of creatine, and it is shown that the technique can obtain solution concentrations to within 7% or better.

  12. Spin orbital theory for the high temperature magnetic phase transitions in Yttrium orthovanadate

    NASA Astrophysics Data System (ADS)

    de Silva, Theja; Joshi, Anuvrat; Zhang, Fu Chun; Ma, Michael

    2003-03-01

    Motivated by recent diffraction experiments, we develope a theoritical model for Yttrium orthovanadate(YVO_3). The key parameters governing the system are on-site coulomb repulsion, Hund's coupling, crystal field splitting between 3d levels and hopping amplitude between nearest neighbor ions. Then, we use a mean field theory to illustrate the relevent physics of the system and verify the existence of the high temperature G-type orbital transition before C-type spin ordering at a lower temperature.

  13. Global calculations of microscopic energies and nuclear deformations: Isospin dependence of the spin-orbit coupling

    NASA Astrophysics Data System (ADS)

    Wu, Zhe-Ying; Qi, Chong; Wyss, Ramon; Liu, Hong-Liang

    2015-08-01

    Background: The deviation between different model calculations that may occur when one goes toward regions where the masses are unknown is getting increased attention. This is related to the uncertainties of the different models which may have not been fully understood. Purpose: To explore in detail the effect of the isospin dependence of the spin-orbital force in the Woods-Saxon potential on global binding energy and deformation calculations. Method: The microscopic energies and nuclear deformations of about 1850 even-even nuclei are calculated systematically within the macroscopic-microscopic framework using three Woods-Saxon parametrizations, with different isospin dependencies, which were constructed mainly for nuclear spectroscopy calculations. Calculations are performed in the deformation space (β2,γ ,β4) . Both the monopole and doubly stretched quadrupole interactions are considered for the pairing channel. Results: The ground-state deformations obtained by the three calculations are quite similar to each other. Large differences are seen mainly in neutron-rich nuclei and in superheavy nuclei. Systematic calculations on the shape-coexisting second minima are also presented. As for the microscopic energies of the ground states, the results are also very close to each other. Only in a few cases the difference is larger than 2 MeV. The total binding energy is estimated by adding the macroscopic energy provided by the usual liquid drop model with its parameters fitted through the least square root and minimax criteria. Calculations are also compared with the results of other macroscopic-microscopic mass models. Conclusions: All the three calculations give similar values for the deformations, microscopic energies, and binding energies of most nuclei. One may expect to have a better understanding of the isospin dependence of the spin-orbital force with more data on proton- and neutron-rich nuclei.

  14. Satellite transitions acquired in real time by magic angle spinning (STARTMAS): ``Ultrafast'' high-resolution MAS NMR spectroscopy of spin I =3/2 nuclei

    NASA Astrophysics Data System (ADS)

    Thrippleton, Michael J.; Ball, Thomas J.; Wimperis, Stephen

    2008-01-01

    The satellite transitions acquired in real time by magic angle spinning (STARTMAS) NMR experiment combines a train of pulses with sample rotation at the magic angle to refocus the first- and second-order quadrupolar broadening of spin I =3/2 nuclei in a series of echoes, while allowing the isotropic chemical and quadrupolar shifts to evolve. The result is real-time isotropic NMR spectra at high spinning rates using conventional MAS equipment. In this paper we describe in detail how STARTMAS data can be acquired and processed with ease on commercial equipment. We also discuss the advantages and limitations of the approach and illustrate the discussion with numerical simulations and experimental data from four different powdered solids.

  15. EDITORIAL: New materials with high spin polarization: half-metallic Heusler compounds

    NASA Astrophysics Data System (ADS)

    Felser, Claudia; Hillebrands, Burkard

    2007-03-01

    dependence of these thin epitaxial Co2FeSi (110) films was investigated using XMCD by Kallmayer et al. The magnetic moment as a function of film thickness demonstrates the presence of dead layers, reducing the magnetization and the spin polarization of these films at all interfaces. The influence of Ga+ ion irradiation was studied using the longitudinal (LMOKE) and quadratic (QMOKE) magneto-optical Kerr effect in a paper by Hamrle et al who, in a second paper, report an unusual huge quadratic magneto-optical Kerr effect in CFS films with L21 structure. The films exhibit a huge QMOKE signal, with its maxima of up to 30 mdeg, which is the largest QMOKE signal in reflection that has been measured thus far. Beside the half-metallicity and the high Curie temperature, an essential feature for such devices is the micro-magnetic domain structure. XMCD-PEEM has been used for a direct observation of the domain structure of single- and polycrystalline samples by Gloskowskii et al. The spin polarization of Co2FeSi films can be improved at room temperature, especially the temperature dependence of the magneto-resistance effect. For a TMR device with Co2FeSi0.5Al0.5 Tezuka et al [3] have found a record TMR value for room temperature. Fecher et al have investigated the electronic structure of Co2FeSi1 - xAlx. The series Co2FeSi1 - xAlx is found to exhibit half-metallic ferromagnetism and it is shown that the electron-doping stabilizes the gap in the minority states for x = 0.5. This might be a reason for the exceptional temperature behavior of Co2FeSi0.5Al0.5 TMR devices. Co2Fe0.5Mn0.5Si is another candidate with Fermi energy in the middle of the minority states gap. Therefore Fecher et al have investigated the electronic structure of the series Co2Fe1 - xMnxSi by high energy, high resolution photoelectron spectroscopy. High energy photoemission is a new advanced method to study the electronic structure of bulk material, due to a large mean free path of the photo electrons. The high

  16. Pure collective precession motion of a high-spin torus isomer

    NASA Astrophysics Data System (ADS)

    Ichikawa, T.; Matsuyanagi, K.; Maruhn, J. A.; Itagaki, N.

    2014-01-01

    We investigate the precession motion of the exotic torus configuration in high-spin excited states of 40Ca. For this aim, we use the three-dimensional time-dependent Hartree-Fock (TDHF) method. Although the high-spin torus isomer is a unique quantum object characterized by the alignment of angular momenta of independent single-particle motions, we find that the obtained moment of inertia for rotations about an axis perpendicular to the symmetry axis is close to the rigid-body value. We also analyze the microscopic structure of the precession motion using the random-phase approximation (RPA) method for high-spin states. In the RPA calculation, the precession motion of the torus isomer is generated by coherent superposition of many one-particle-one-hole excitations across the sloping Fermi surface that strongly violates the time-reversal symmetry. By comparing results of the TDHF and the RPA calculations, we find that the precession motion obtained by the TDHF calculation is a pure collective motion well decoupled from other collective modes.

  17. Spin-orbital nature of the high-field magnetic state in the Sr4Ru3O10

    NASA Astrophysics Data System (ADS)

    Granata, Veronica; Capogna, Lucia; Forte, Filomena; Lepetit, Marie-Bernadette; Fittipaldi, Rosalba; Stunault, Anne; Cuoco, Mario; Vecchione, Antonio

    2016-03-01

    We perform a spin-polarized neutron-diffraction study to investigate the nature of the high-field magnetic state of the trilayered Sr4Ru3O10 . The analysis indicates that a high field applied within the a b plane leads to an unbalance of the spin and orbital moments with a spatial profile that is strongly tied to the layers where the electrons are located in the unit cell. We provide evidence of a layer dependent magnetic anisotropy with the inner layers having larger spin and orbital magnetic moments than the outer ones and show that such behavior is robust to temperature variation being persistent above the Curie temperature. By means of an effective model that includes the coupling between the spin-orbital degrees of freedom at inequivalent Ru sites we ascribe the origin of the layer anisotropy to the cooperative effects between octahedral distortions, spin orbit, and Coulomb interactions.

  18. Pure spin current in lateral structures

    NASA Astrophysics Data System (ADS)

    Chen, Shuhan

    Spintronics, a frontier academic research area, is advancing rapidly in recent years. It has been chosen as one of the promising candidates for overcoming the obstacles in continuing the "Moore's Law" of the electronics industry. Spintronics employs both spin and charge degrees of freedom of electrons to reduce energy consumption and increase the flexibility of IC design. To achieve this, it is extremely important to understand the generation, transport, and detection of the spin polarized current (spin current). In this work we use a mesoscopic metallic spintronic structure-nonlocal spin valve (NLSV)-for fundamental studies of spintronics. A nonlocal spin valve consists of two ferromagnetic electrodes (a spin injector and a spin detector) bridged by a non-magnetic spin channel. A thin aluminum oxide barrier (~ 2 - 3 nm) has been shown to effectively enhance the spin injection and detection polarizations. We have studied spin injection and detection in these nanoscale structures. Several topics will be discussed in this work. In Chapter 4 we explore spin transport in NLSVs with Ag channels. Substantial spin signals are observed. The temperature dependence of the spin signals indicates long spin diffusion lengths and low surface spin-flip rate in the mesoscopic Ag channels. Chapter 5 will focus on the asymmetric spin absorption across the low-resistance AlOx barriers in NLSVs. This effect allows for a more simplified and efficient detection scheme for the spin accumulation. Then in Chapter 6 we report a large spin signal owing to a highly resistive break-junction. We have also developed a model to describe the spin-charge coupling effect which enables the large spin signal. In the end, Spin Hall Effect (SHE) is investigated in Chapter 7. A mesoscopic Pt film is utilized to inject a spin accumulation into a mesoscopic Cu channel via the SHE. The spin accumulation in Cu can be detected by the nonlocal method. The reciprocal effect -- the inverse Spin Hall Effect - (i

  19. High-energy neutron dosimetry

    NASA Astrophysics Data System (ADS)

    Sutton, Michele Rhea

    2001-12-01

    Fluence-to-dose conversion coefficients for the radiation protection quantity effective dose were calculated for neutrons, photons and protons with energies up to 2 GeV using the MCNPX code. The calculations were performed using the Pacific Northwest National Laboratory versions of the MIRD-V male and female anthropomorphic phantoms modified to include the skin and esophagus. The latest high-energy neutron evaluated cross-section libraries and the recommendations given in ICRP Publication 60 and ICRP Publication 74 were utilized to perform the calculations. Sets of fluence-to- effective dose conversion coefficients are given for anterior-posterior, posterior-anterior, left-lateral, right-lateral and rotational irradiation geometries. This is the first set of dose conversion coefficients over this energy range calculated for the L-LAT irradiation geometry. A unique set of high-energy neutron depth-dose benchmark experiments were performed at the Los Alamos Neutron Science Center/Weapons Neutron Research (LANSCE/WNR) complex. The experiments consisted of filtered neutron beams with energies up to 800 MeV impinging on a 30 x 30 x 30 cm3 tissue-equivalent phantom. The absorbed dose was measured in the phantom at various depths with tissue-equivalent ion chambers. The phantom and the experimental set-up were modeled using MCNPX. Comparisons of the experimental and computational depth- dose distributions indicate that the absorbed dose calculated by MCNPX is within 13% for neutrons with energies up to 750 MeV. This experiment will serve as a benchmark experiment for the testing of high-energy radiation transport codes for the international radiation protection community.

  20. One-loop correction to the energy of spinning strings in S{sup 5}

    SciTech Connect

    Frolov, S.A.; Park, I.Y.; Tseytlin, A.A.

    2005-01-15

    We revisit the computation of the 1-loop AdS{sub 5}xS{sup 5} superstring sigma model correction to the energy of a closed circular string rotating in S{sup 5}. The string is spinning around its center of mass with two equal angular momenta J{sub 2}=J{sub 3} and its center of mass angular momentum is J{sub 1}. We revise the argument that the 1-loop correction is suppressed by (1/J) factor [J=J{sub 1}+2J{sub 2} is the total SO(6) spin] relative to the classical ({lambda}J{sub 2}/J{sup 2}) term in the energy and use numerical methods to compute the leading 1-loop coefficient. The corresponding gauge-theory result is known only in the J{sub 1}=0 limit when the string solution becomes unstable and thus the 1-loop shift of the energy formally contains an imaginary part. While the comparison with gauge-theory may not be well defined in this case, our numerical string-theory value of the 1-loop coefficient seems to disagree with the gauge-theory one. A plausible explanation should be in the different order of limits taken on the gauge-theory and the string-theory sides of the anti-de Sitter/conformal field theory duality.

  1. High energy gamma ray astronomy

    NASA Technical Reports Server (NTRS)

    Fichtel, Carl E.

    1987-01-01

    High energy gamma ray astronomy has evolved with the space age. Nonexistent twenty-five years ago, there is now a general sketch of the gamma ray sky which should develop into a detailed picture with the results expected to be forthcoming over the next decade. The galactic plane is the dominant feature of the gamma ray sky, the longitude and latitude distribution being generally correlated with galactic structural features including the spiral arms. Two molecular clouds were already seen. Two of the three strongest gamma ray sources are pulsars. The highly variable X-ray source Cygnus X-3 was seen at one time, but not another in the 100 MeV region, and it was also observed at very high energies. Beyond the Milky Way Galaxy, there is seen a diffuse radiation, whose origin remains uncertain, as well as at least one quasar, 3C 273. Looking to the future, the satellite opportunities for high energy gamma ray astronomy in the near term are the GAMMA-I planned to be launched in late 1987 and the Gamma Ray Observatory, scheduled for launch in 1990. The Gamma Ray Observatory will carry a total of four instruments covering the entire energy range from 30,000 eV to 3 x 10 to the 10th eV with over an order of magnitude increase in sensitivity relative to previous satellite instruments.

  2. High energy density electrochemical cell

    NASA Technical Reports Server (NTRS)

    Byrne, J. J.; Williams, D. L.

    1970-01-01

    Primary cell has an anode of lithium, a cathode containing dihaloisocyanuric acid, and a nonaqueous electrolyte comprised of a solution of lithium perchlorate in methyl formate. It produces an energy density of 213 watt hrs/lb and can achieve a high current density.

  3. Nuclear magnetic resonance-paramagnetic relaxation enhancements: Influence of spatial quantization of the electron spin when the zero-field splitting energy is larger than the Zeeman energy

    NASA Astrophysics Data System (ADS)

    Abernathy, S. M.; Miller, J. C.; Lohr, L. L.; Sharp, R. R.

    1998-09-01

    Dissolved paramagnetic ions generally provide an efficient mechanism for the relaxation of nuclear spins in solution, a phenomenon called the nuclear magnetic resonance-paramagnetic relaxation enhancement (NMR-PRE). Metal ions with electron spins S⩾1 exhibit rich NMR relaxation phenomena originating in the properties of the zero-field splitting (zfs) interaction, which vanishes for spin-1/2 ions but which is nonzero for S⩾1 ions in site symmetry lower than cubic. For S⩾1 ions in the vicinity of the zfs-limit, i.e., at magnetic-field strengths low enough that the zfs energy exceeds the Zeeman energy, the NMR-PRE depends strongly on the detailed structure of the electron spin energy levels as well as on the spatial quantization of the spin motion. It is shown theoretically and experimentally that the NMR-PRE produced by integer spins can be influenced strongly by the small intradoublet zero-field splittings, i.e., the splittings between the components of the non-Kramers doublets, which are produced by noncylindrical components of the crystal field potential. These small splittings produce relatively low-frequency oscillations in the dipolar field associated with (the spin component along the molecule-fixed ẑ axis). These motions decouple the nuclear spin from the electron spin, thereby depressing, in some cases very strongly, the NMR-PRE. The presence of a relatively small Zeeman field, comparable in magnitude to the intradoublet spacing but small compared to the larger interdoublet zfs splittings, causes a major change in the spin wave functions which has profound effects on the motions of the electron spin. When the Zeeman energy exceeds the small zfs splitting, the oscillatory motion of damps out, with the result that the electron spin couples more effectively to the nuclear spin, providing a more efficient NMR relaxation pathway. NMR-PRE data are presented for the S=1 complex Ni(II)(o-pda)2Cl2 (o-pda=ortho-phenylenediamine) which confirm the

  4. RF-SABRE: A Way to Continuous Spin Hyperpolarization at High Magnetic Fields.

    PubMed

    Pravdivtsev, Andrey N; Yurkovskaya, Alexandra V; Vieth, Hans-Martin; Ivanov, Konstantin L

    2015-10-29

    A new technique is developed that allows one to carry out the signal amplification by reversible exchange (SABRE) experiments at high magnetic field. SABRE is a hyperpolarization method, which utilizes transfer of spin order from para-hydrogen to the spins of a substrate in transient iridium complexes. Previously, it has been thought that such a transfer of spin order is only efficient at low magnetic fields, notably, at level anti-crossing (LAC) regions. Here it is demonstrated that LAC conditions can also be fulfilled at high fields under the action of a RF field. The high-field RF-SABRE experiment can be implemented using commercially available nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) machines and does not require technically demanding field-cycling. The achievable NMR enhancements are around 100 for several substrates as compared to their NMR signals at thermal equilibrium conditions at 4.7 T. The frequency dependence of RF-SABRE is comprised of well pronounced peaks and dips, whose position and amplitude are conditioned solely by the magnetic resonance parameters such as chemical shifts and scalar coupling of the spin system involved in the polarization transfer and by the amplitude of the RF field. Thus, the proposed method can serve as a new sensitive tool for probing transient complexes. Simulations of the dependence of magnetization transfer (i.e., NMR signal amplifications) on the frequency and amplitude of the RF field are in good agreement with the developed theoretical approach. Furthermore, the method enables continuous re-hyperpolarization of the SABRE substrate over a long period of time, giving a straightforward way to repetitive NMR experiments. PMID:25970807

  5. Spin-spin and spin-orbit interaction effects of two-electron quantum dots

    NASA Astrophysics Data System (ADS)

    Vaseghi, B.; Rezaei, G.; Taghizadeh, S. F.; Shahedi, Z.

    2014-09-01

    Simultaneous effects of spin-spin and spin-orbit interactions on the energy spectrum of a two-electron spherical quantum dot with parabolic confinement and under the influence of external electric and magnetic fields are investigated. We have calculated energy eigenvalues and eigenvectors of the system for different spin states. Results show that effects of spin-spin interactions are negligible in comparison with those of the spin-orbit interactions. Spin-orbit interaction splits energy levels and removes degeneracy of different spin states. Moreover it is seen that energy eigenvalues and levels splitting strongly depend on the external magnetic field and the dot dimensions.

  6. Mononuclear Nonheme High-Spin (S=2) versus Intermediate-Spin (S=1) Iron(IV)-Oxo Complexes in Oxidation Reactions.

    PubMed

    Bae, Seong Hee; Seo, Mi Sook; Lee, Yong-Min; Cho, Kyung-Bin; Kim, Won-Suk; Nam, Wonwoo

    2016-07-01

    Mononuclear nonheme high-spin (S=2) iron(IV)-oxo species have been identified as the key intermediates responsible for the C-H bond activation of organic substrates in nonheme iron enzymatic reactions. Herein we report that the C-H bond activation of hydrocarbons by a synthetic mononuclear nonheme high-spin (S=2) iron(IV)-oxo complex occurs through an oxygen non-rebound mechanism, as previously demonstrated in the C-H bond activation by nonheme intermediate (S=1) iron(IV)-oxo complexes. We also report that C-H bond activation is preferred over C=C epoxidation in the oxidation of cyclohexene by the nonheme high-spin (HS) and intermediate-spin (IS) iron(IV)-oxo complexes, whereas the C=C double bond epoxidation becomes a preferred pathway in the oxidation of deuterated cyclohexene by the nonheme HS and IS iron(IV)-oxo complexes. In the epoxidation of styrene derivatives, the HS and IS iron(IV) oxo complexes are found to have similar electrophilic characters. PMID:27273456

  7. Production of the (I = 19/2) high-spin isomer {sup 135}Cs in photonuclear reactions

    SciTech Connect

    Gangrsky, Yu. P.; Zhemenik, V. I.; Kolesnikov, N. N.; Lukashik, V. G.; Markov, B. N.; Myshinskiy, G. V.; Maslov, O. D.; Bozhikov, G. A.

    2010-09-15

    The yields of {sup 135}Cs nuclei in a high-spin (19/2) isomeric state and of nuclei neighboring it were measured for photonuclear reactions of the ({gamma}, f) and ({gamma}, {alpha}) types. The experiments in question were performed by using bremsstrahlung from a microtron at the maximum electron energy of 25 MeV. The product nuclei were identified by their half-lives and by the lines of gamma radiation emitted in their decay, and the reaction yields R were determined by the ratios of the intensities of these lines to the bremsstrahlung flux. The cross sections for isomer production were calculated, and the angular momenta of product nuclei immediately before the cascade of gamma transitions populating the ground or an isomeric nuclear state were evaluated on the basis of these results. An enhanced yield of the high-spin isomer of {sup 135}Cs in the fission reaction in relation to the respective ({gamma}, {alpha}) reaction and in relation to the results of the calculations is found.

  8. Accurate potential energy functions, non-adiabatic and spin-orbit couplings in the ZnH+ system

    NASA Astrophysics Data System (ADS)

    Liang, Guiying; Liu, Xiaoting; Zhang, Xiaomei; Xu, Haifeng; Yan, Bing

    2016-03-01

    A high-level ab initio calculation on the ZnH+ cation has been carried out with the multi-reference configuration interaction method plus Davison correction (MRCI + Q). The scalar relativistic effect is included by using the Douglas-Kroll-Hess (DKH) method. The calculated potential energy curves (PECs) of the 7 Λ-S states are associated with the dissociation limits of Zn+(2Sg) + H(2Sg), Zn(1Sg) + H+(1Sg), and Zn+(2Pu) + H(2Sg), respectively (The Λ-S state is labeled as 2S + 1Λ, in which Λ is the quantum number for the projection along the internuclear axis of the total electronic orbital angular momentum and S is the total electron spin). The spectroscopic constants of the bound states are determined and in good agreement with the available theoretical and experimental results. The permanent dipole moments (PDMs) of Λ-S states and the spin-orbit (SO) matrix elements between Λ-S states are also computed. The results show that the abrupt changes of the PDMs and SO matrix elements come into being for the reason of the avoided crossing between the states with the same symmetry. In addition, the non-adiabatic couplings matrix elements between Λ-S states are also evaluated. Finally, the spin-orbit couplings (SOCs) for the low-lying states are considered with Breit-Pauli operator. The SOC effect makes the 7 Λ-S states of the ZnH+ cation split into 12 Ω states (Ω = Λ + Sz, in which Sz is projection of the total electron spin S along the internuclear Z-axis). For the (3)0+ state, the two energy minima exhibit in the potential, which could be attributed to the formation of the new avoided crossing point. The transition dipole moments (TDMs), Franck-Condon factors, and the radiative lifetimes of the selected transitions (2)0+-X0+, (3)0+-X0+, (2)1-X0+ and (3)1-X0+ have been reported.

  9. Accurate potential energy functions, non-adiabatic and spin-orbit couplings in the ZnH(+) system.

    PubMed

    Liang, Guiying; Liu, Xiaoting; Zhang, Xiaomei; Xu, Haifeng; Yan, Bing

    2016-03-01

    A high-level ab initio calculation on the ZnH(+) cation has been carried out with the multi-reference configuration interaction method plus Davison correction (MRCI+Q). The scalar relativistic effect is included by using the Douglas-Kroll-Hess (DKH) method. The calculated potential energy curves (PECs) of the 7 Λ-S states are associated with the dissociation limits of Zn(+)((2)Sg)+H((2)Sg), Zn((1)Sg)+H(+)((1)Sg), and Zn(+)((2)Pu)+H((2)Sg), respectively (The Λ-S state is labeled as (2S+1)Λ, in which Λ is the quantum number for the projection along the internuclear axis of the total electronic orbital angular momentum and S is the total electron spin). The spectroscopic constants of the bound states are determined and in good agreement with the available theoretical and experimental results. The permanent dipole moments (PDMs) of Λ-S states and the spin-orbit (SO) matrix elements between Λ-S states are also computed. The results show that the abrupt changes of the PDMs and SO matrix elements come into being for the reason of the avoided crossing between the states with the same symmetry. In addition, the non-adiabatic couplings matrix elements between Λ-S states are also evaluated. Finally, the spin-orbit couplings (SOCs) for the low-lying states are considered with Breit-Pauli operator. The SOC effect makes the 7 Λ-S states of the ZnH(+) cation split into 12 Ω states (Ω=Λ+Sz, in which Sz is projection of the total electron spin S along the internuclear Z-axis). For the (3)0(+) state, the two energy minima exhibit in the potential, which could be attributed to the formation of the new avoided crossing point. The transition dipole moments (TDMs), Franck-Condon factors, and the radiative lifetimes of the selected transitions (2)0(+)-X0(+), (3)0(+)-X0(+), (2)1-X0(+) and (3)1-X0(+) have been reported. PMID:26637984

  10. High field 207Pb spin-lattice relaxation in solid lead nitrate and lead molybdate

    NASA Astrophysics Data System (ADS)

    de Castro, Peter J.; Maher, Christopher A.; Vold, Robert L.; Hoatson, Gina L.

    2008-02-01

    Spin-lattice relaxation rates of lead have been measured at 17.6T (156.9MHz) as a function of temperature in polycrystalline lead nitrate and lead molybdate. Comparing the results with relaxation rates measured at lower fields, it is found that at high fields and low temperature, chemical shift anisotropy (CSA) makes small but observable contributions to lead relaxation in both materials. At 17.6T and 200K, CSA accounts for about 15% of the observed relaxation rate. Above 300K, the dominant relaxation mechanism even at 17.6T is an indirect Raman process involving modulation of the Pb207 spin-rotation tensor, as first proposed by Grutzner et al. [J. Am. Chem. Soc. 123, 7094 (2001)] and later treated theoretically in more detail by Vega et al. [Phys. Rev. B 74, 214420 (2006)]. The improved signal to noise ratio at high fields makes it possible to quantify relaxation time anisotropy by analyzing saturation-recovery functions for individual frequencies on the powder pattern line shape. No orientation dependence is found for the spin-lattice relaxation rate of either material. It is argued from examination of the appropriate theoretical expressions, derived here for the first time, that the lack of observable relaxation time anisotropy is probably a general feature of this indirect Raman mechanism.

  11. High spin structure of the neutron-rich nuclei {sup 137}I and {sup 139}Cs

    SciTech Connect

    Liu, S. H.; Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Covello, A.; Itaco, N.; Gargano, A.; Luo, Y. X.; Rasmussen, J. O.; Daniel, A. V.; Ter-Akopian, G. M.; Zhu, S. J.; Ma, W. C.

    2009-10-15

    High spin excited states in the neutron-rich nuclei {sup 137}I and {sup 139}Cs were investigated from a study of the prompt {gamma} rays emitted in the spontaneous fission of {sup 252}Cf with the Gammasphere detector array. Ten new excited levels with 18 new deexciting transitions were observed in {sup 139}Cs and the level scheme of {sup 139}Cs was extended up to 4670 keV. Spins and parities of levels in {sup 139}Cs were firmly assigned up to 25/2{sup +}. Three new levels were found in {sup 137}I. Shell model calculations were performed to interpret the experimental results. A good agreement between theory and experiment in both nuclei was found.

  12. Room temperature high-fidelity holonomic single-qubit gate on a solid-state spin

    PubMed Central

    Arroyo-Camejo, Silvia; Lazariev, Andrii; Hell, Stefan W.; Balasubramanian, Gopalakrishnan

    2014-01-01

    At its most fundamental level, circuit-based quantum computation relies on the application of controlled phase shift operations on quantum registers. While these operations are generally compromised by noise and imperfections, quantum gates based on geometric phase shifts can provide intrinsically fault-tolerant quantum computing. Here we demonstrate the high-fidelity realization of a recently proposed fast (non-adiabatic) and universal (non-Abelian) holonomic single-qubit gate, using an individual solid-state spin qubit under ambient conditions. This fault-tolerant quantum gate provides an elegant means for achieving the fidelity threshold indispensable for implementing quantum error correction protocols. Since we employ a spin qubit associated with a nitrogen-vacancy colour centre in diamond, this system is based on integrable and scalable hardware exhibiting strong analogy to current silicon technology. This quantum gate realization is a promising step towards viable, fault-tolerant quantum computing under ambient conditions. PMID:25216026

  13. Odd tensor electric transitions in high-spin Sn-isomers and generalized seniority

    NASA Astrophysics Data System (ADS)

    Maheshwari, Bhoomika; Jain, Ashok Kumar

    2016-02-01

    The similar behavior of the B (E 1) values of the recently observed 13- odd tensor E1 isomers and the B (E 2) values of the 10+ and 15- even tensor E2 isomers in the Sn-isotopes has been understood in terms of the generalized seniority for multi-j orbits by using the quasi-spin scheme. This simple approach proves to be quite successful in explaining the measured transition probabilities and the corresponding half-lives in the high-spin isomers of the semi-magic Sn-isotopes. Hence, we show for the first time the occurrence of seniority isomers in the 13- Sn-isomers, which decay by odd-tensor E1 transitions to the same seniority states.

  14. High-temperature heat capacity of Co3O4 spinel: thermally induced spin unpairing transition

    USGS Publications Warehouse

    Mocala, K.; Navrotsky, A.; Sherman, David M.

    1992-01-01

    A strong anomaly was found in the heat capacity of Co3O4 between 1000 K and the decomposition temperature. This anomaly is not related to the decomposition of Co3O4 to CoO. The measured entropy of transition, ??S=46??4 J mol-1 K-1 of Co3O4, supports the interpretation that this anomaly reflects a spin unpairing transition in octahedrally coordinated Co3+ cations. Experimental values of heat capacity, heat content and entropy of Co3O4 in the high temperature region are provided. The enthalpy of the spin unpairing transition is 53??4 kJ mol-1 of Co3O4. ?? 1992 Springer-Verlag.

  15. Nonlinear magnetic field dependence of spin polarization in high-density two-dimensional electron systems

    NASA Astrophysics Data System (ADS)

    Yang, K. F.; Liu, H. W.; Mishima, T. D.; Santos, M. B.; Nagase, K.; Hirayama, Y.

    2011-08-01

    The spin polarization (P) of high-density InSb two-dimensional electron systems (2DESs) has been measured using both parallel and tilted magnetic fields. P is found to exhibit a superlinear increase with the total field B. This P-B nonlinearity results in a difference in spin susceptibility between its real value χs and χgm~ m*g* (m* and g* are the effective mass and g factor, respectively) as routinely used in experiments. We demonstrate that such a P-B nonlinearity originates from the linearly P-dependent g* due to the exchange coupling of electrons rather than from the electron correlation as predicted for the low-density 2DES.

  16. Room temperature high-fidelity holonomic single-qubit gate on a solid-state spin.

    PubMed

    Arroyo-Camejo, Silvia; Lazariev, Andrii; Hell, Stefan W; Balasubramanian, Gopalakrishnan

    2014-01-01

    At its most fundamental level, circuit-based quantum computation relies on the application of controlled phase shift operations on quantum registers. While these operations are generally compromised by noise and imperfections, quantum gates based on geometric phase shifts can provide intrinsically fault-tolerant quantum computing. Here we demonstrate the high-fidelity realization of a recently proposed fast (non-adiabatic) and universal (non-Abelian) holonomic single-qubit gate, using an individual solid-state spin qubit under ambient conditions. This fault-tolerant quantum gate provides an elegant means for achieving the fidelity threshold indispensable for implementing quantum error correction protocols. Since we employ a spin qubit associated with a nitrogen-vacancy colour centre in diamond, this system is based on integrable and scalable hardware exhibiting strong analogy to current silicon technology. This quantum gate realization is a promising step towards viable, fault-tolerant quantum computing under ambient conditions. PMID:25216026

  17. Macroscopic Measurement of Resonant Magnetization Tunneling in High-Spin Molecules

    NASA Astrophysics Data System (ADS)

    Friedman, Jonathan R.; Sarachik, M. P.; Tejada, J.; Maciejewski, J.; Ziolo, R.

    1996-03-01

    We report the observation of steps in the hysteresis loop of a macroscopic sample of oriented crystals of Mn_12O_12(CH_3COO)_16(H_2O)_4, a high-spin (S=10) molecule. The steps occur at regular intervals of magnetic field, every 0.46 T. The magnetic relaxation rate increases substantially when the field is tuned to a step. We interpret these effects as manifestations of thermally assisted, field-tuned resonant tunneling between quantum spin states. A simple model is presented that accounts for the observations and yields good quantitative agreement with measured values of the anisotropy barrier. We attribute the observation of quantum-mechanical phenomena on a macroscopic scale to tunneling in a large (Avogadro's) number of magnetically identical molecules.

  18. Ab initio Potential-Energy Surfaces and Electron-Spin-Exchange Cross Sections for H-O2 Interactions

    NASA Technical Reports Server (NTRS)

    Stallcop, James R.; Partridge, Harry; Levin, Eugene

    1996-01-01

    Accurate quartet- and doublet-state potential-energy surfaces for the interaction of a hydrogen atom and an oxygen molecule in their ground states have been determined from an ab initio calculation using large-basis sets and the internally contracted multireference configuration interaction method. These potential surfaces have been used to calculate the H-O2 electron-spin-exchange cross section; the square root of the cross section (in a(sub 0)), not taking into account inelastic effects, can be obtained approximately from the expressions 2.390E(sup -1/6) and 5.266-0.708 log10(E) at low and high collision energies E (in E(sub h)), respectively. These functional forms, as well as the oscillatory structure of the cross section found at high energies, are expected from the nature of the interaction energy. The mean cross section (the cross section averaged over a Maxwellian velocity distribution) agrees reasonably well with the results of measurements.

  19. CRYSTALLINE BEAMS AT HIGH ENERGIES.

    SciTech Connect

    WEI, J.; OKAMOTO, H.; YURI, Y.; SESSLER, A.; MACHIDA, S.

    2006-06-23

    Previously it was shown that by crystallizing each of the two counter-circulating beams, a much larger beam-beam tune shift can be tolerated during the beam-beam collisions; thus a higher luminosity can be reached for colliding beams [1]. On the other hand, crystalline beams can only be formed at energies below the transition energy ({gamma}{sub T}) of the accelerators [2]. In this paper, we investigate the formation of crystals in a high-{gamma}{sub T} lattice that also satisfies the maintenance condition for a crystalline beam [3].

  20. Spin and orbital magnetic moments and spin anisotropy energies of light rare earth atoms embedded in graphene: A first-principles study

    NASA Astrophysics Data System (ADS)

    Li, Ya-Jing; Wang, Min; Tang, Meng-yu; Tian, Xing; Gao, Shan; He, Zhen; Li, Ying; Zhou, Tie-Ge

    2016-01-01

    The geometries, electronic structures, spin magnetic moments (SMMs), orbital magnetic moments (OMMs) and spin anisotropy energies (SAEs) of light rare earth atoms (La, Ce, Pr, Nd, Pm, Sm, Eu, and Gd) embedded in graphene were studied by using first-principles calculations based on Density Functional Theory (DFT). The spin-orbital coupling effect was taken into account and GGA+U method was adopted to describe the strongly localized and correlated 4f electrons. There is a significant deformation of the graphene plane after doping and optimization. The deformation of Gd doped graphene is the largest, while Eu the smallest. The results show that the valence is +3 for La, Ce, Pr, Nd, Pm, Sm and Gd, and +2 for Eu. Except Eu and Gd, there are obvious OMMs. When the spin is in the Z direction, the OMMs are -0.941 μB, -1.663 μB, -3.239 μB, -3.276 μB and -3.337 μB for Ce, Pr, Nd, Pm and Sm, respectively, and point the opposite direction of SMMs. All the doped systems except Gd show considerable SAEs. For Ce, Pr, Nd, Pm, Sm, and Eu, the SAEs are -0.928 meV, 20.941 meV, -8.848 meV, 7.855 meV, 75.070 meV and 0.810 meV, respectively. When the spin orientation is different, different orbital angular moments lead to apparent charge density difference of the 4f atoms, which can also explain the origin of SAEs.