Science.gov

Sample records for low-background gamma spectroscopy

  1. Applications of the low-background gamma spectroscopy to the geographical origin of marine salts and prunes

    SciTech Connect

    Perrot, F.

    2007-03-28

    The low background gamma spectroscopy has been applied to try to sign the geographical origin of the French atlantic marine salts and of the prunes from Agen. Most of the activity measurements have been done using low background Ge spectrometers located in Bordeaux. Results have shown that a clear signature exists in the case of the French atlantic salts using the 40K, 137Cs and 226Ra isotopes but not in the case of the prunes.

  2. The Dortmund Low Background Facility - Low-background gamma ray spectrometry with an artificial overburden.

    PubMed

    Gastrich, Holger; Gößling, Claus; Klingenberg, Reiner; Kröninger, Kevin; Neddermann, Till; Nitsch, Christian; Quante, Thomas; Zuber, Kai

    2016-06-01

    The Dortmund Low Background Facility is an instrument for low-level gamma ray spectrometry with an artificial overburden of ten meters of water equivalent, an inner shielding, featuring a neutron absorber, and an active muon veto. An integral background count rate between 40keV and 2700keV of (2.528±0.004)counts/(kgmin) enables low-background gamma ray spectrometry with sensitivities in the range of some 10mBq/kg within a week of measurement time. PMID:27082973

  3. Low Background Gamma-Ray Spectrometry in the 'Laboratoire Souterrain de Modane'

    SciTech Connect

    Hubert, Ph.; Hubert, F.

    2007-03-28

    Most of the underground experiments in physics and many studies in geology, biology or environmental sciences face a common requirement with the necessity of using experimental devices with ultra-low background radioactivity. Many developments involving many different techniques have been used in order to be able to measure extremely low levels of radioactivity in materials. This report will focus on low background gamma-ray spectrometry and will describe the work which has been carried out over the last fifteen years in the 'Laboratoire Souterrain de Modane' (LSM)

  4. Berkeley Low Background Facility

    NASA Astrophysics Data System (ADS)

    Thomas, K. J.; Smith, A. R.; Poon, A. W. P.; Chan, Y. D.; Norman, E. B.; Lesko, K. T.

    2015-08-01

    The Berkeley Low Background Facility (BLBF) at Lawrence Berkeley National Laboratory (LBNL) in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background laboratory on the surface at LBNL and at the Sanford Underground Research Facility (SURF) in Lead, SD. These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K) or common cosmogenic/anthropogenic products; active screening via neutron activation analysis for U,Th, and K as well as a variety of stable isotopes; and neutron flux/beam characterization measurements through the use of monitors. A general overview of the facilities, services, and sensitivities will be presented. Recent activities and upgrades will also be described including an overview of the recently installed counting system at SURF (recently relocated from Oroville, CA in 2014), the installation of a second underground counting station at SURF in 2015, and future plans. The BLBF is open to any users for counting services or collaboration on a wide variety of experiments and projects.

  5. Berkeley Low Background Facility

    SciTech Connect

    Thomas, K. J.; Norman, E. B.; Smith, A. R.; Poon, A. W. P.; Chan, Y. D.; Lesko, K. T.

    2015-08-17

    The Berkeley Low Background Facility (BLBF) at Lawrence Berkeley National Laboratory (LBNL) in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background laboratory on the surface at LBNL and at the Sanford Underground Research Facility (SURF) in Lead, SD. These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K) or common cosmogenic/anthropogenic products; active screening via neutron activation analysis for U,Th, and K as well as a variety of stable isotopes; and neutron flux/beam characterization measurements through the use of monitors. A general overview of the facilities, services, and sensitivities will be presented. Recent activities and upgrades will also be described including an overview of the recently installed counting system at SURF (recently relocated from Oroville, CA in 2014), the installation of a second underground counting station at SURF in 2015, and future plans. The BLBF is open to any users for counting services or collaboration on a wide variety of experiments and projects.

  6. Application of low-background gamma-ray spectrometry to monitor radioactivity in the environment and food.

    PubMed

    Khan, A J; Semkow, T M; Beach, S E; Haines, D K; Bradt, C J; Bari, A; Syed, U-F; Torres, M; Marrantino, J; Kitto, M E; Menia, T; Fielman, E

    2014-08-01

    The results are described of an upgrade of the low-background gamma-ray spectrometry laboratory at New York State Department of Health by acquiring sensitivity to low-energy gamma rays. Tuning of the spectrometer and its low-energy response characteristics are described. The spectrometer has been applied to monitor the environment by measuring aerosols and water in New York State contaminated by the 2011 Fukushima accident plume. In addition, the spectrometer has been used to monitor radioactivity in food by performing a study of cesium in Florida milk. PMID:24836905

  7. Low Background Counting at LBNL

    DOE PAGESBeta

    Smith, A. R.; Thomas, K. J.; Norman, E. B.; Chan, Y. D.; Lesko, K. T.; Hurley, D. L.

    2015-03-24

    The Low Background Facility (LBF) at Lawrence Berkeley National Laboratory in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background cave and remotely at an underground location that historically has operated underground in Oroville, CA, but has recently been relocated to the Sanford Underground Research Facility (SURF) in Lead, SD. These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K)more » or common cosmogenic/anthropogenic products, as well as active screening via Neutron Activation Analysis for specific applications. The LBF also provides hosting services for general R&D testing in low background environments on the surface or underground for background testing of detector systems or similar prototyping. A general overview of the facilities, services, and sensitivities is presented. Recent activities and upgrades will also be presented, such as the completion of a 3π anticoincidence shield at the surface station and environmental monitoring of Fukushima fallout. The LBF is open to any users for counting services or collaboration on a wide variety of experiments and projects.« less

  8. Low Background Counting at LBNL

    SciTech Connect

    Smith, A. R.; Thomas, K. J.; Norman, E. B.; Chan, Y. D.; Lesko, K. T.; Hurley, D. L.

    2015-03-24

    The Low Background Facility (LBF) at Lawrence Berkeley National Laboratory in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background cave and remotely at an underground location that historically has operated underground in Oroville, CA, but has recently been relocated to the Sanford Underground Research Facility (SURF) in Lead, SD. These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K) or common cosmogenic/anthropogenic products, as well as active screening via Neutron Activation Analysis for specific applications. The LBF also provides hosting services for general R&D testing in low background environments on the surface or underground for background testing of detector systems or similar prototyping. A general overview of the facilities, services, and sensitivities is presented. Recent activities and upgrades will also be presented, such as the completion of a 3π anticoincidence shield at the surface station and environmental monitoring of Fukushima fallout. The LBF is open to any users for counting services or collaboration on a wide variety of experiments and projects.

  9. Low Background Counting at LBNL

    NASA Astrophysics Data System (ADS)

    Smith, A. R.; Thomas, K. J.; Norman, E. B.; Chan, Y. D.; Lesko, K. T.; Hurley, D. L.

    The Low Background Facility (LBF) at Lawrence Berkeley National Laboratory in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background cave and remotely at an underground location that historically has operated underground in Oroville, CA, but has recently been relocated to the Sanford Underground Research Facility (SURF) in Lead, SD. These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K) or common cosmogenic/anthropogenic products, as well as active screening via Neutron Activation Analysis for specific applications. The LBF also provides hosting services for general R&D testing in low background environments on the surface or underground for background testing of detector systems or similar prototyping. A general overview of the facilities, services, and sensitivities is presented. Recent activities and upgrades will also be presented, such as the completion of a 3π anticoincidence shield at the surface station and environmental monitoring of Fukushima fallout. The LBF is open to any users for counting services or collaboration on a wide variety of experiments and projects.

  10. Two-photon fluorescence correlation spectroscopy with high count rates and low background using dielectric microspheres

    PubMed Central

    Aouani, Heykel; Schön, Peter; Brasselet, Sophie; Rigneault, Hervé; Wenger, Jérôme

    2010-01-01

    Two-photon excitation fluorescence is a powerful technique commonly used for biological imaging. However, the low absorption cross section of this non-linear process is a critical issue for performing biomolecular spectroscopy at the single molecule level. Enhancing the two-photon fluorescence signal would greatly improve the effectiveness of this technique, yet current methods struggle with medium enhancement factors and/or high background noise. Here, we show that the two-photon fluorescence signal from single Alexa Fluor 488 molecules can be enhanced up to 10 times by using a 3 µm diameter latex sphere while adding almost no photoluminescence background. We report a full characterization of the two-photon fluorescence enhancement by a single microsphere using fluorescence correlation spectroscopy. This opens new routes to enhance non-linear optical signals and extend biophotonic applications. PMID:21258531

  11. Low-Background In-Trap Decay Spectroscopy with TITAN at TRIUMF

    NASA Astrophysics Data System (ADS)

    Leach, K. G.; Lennarz, A.; Grossheim, A.; Klawitter, R.; Brunner, T.; Chaudhuri, A.; Chowdhury, U.; Crespo López-Urrutia, J. R.; Gallant, A. T.; Kwiatkowski, A. A.; Macdonald, T. D.; Schultz, B. E.; Seeraji, S.; Andreoiu, C.; Frekers, D.; Dilling, J.

    An in-trap decay spectroscopy setup has been developed and constructed for use with the TITAN facility at TRIUMF. The goal of this device is to observe weak electron-capture (EC) branching ratios for the odd-odd intermediate nuclei in the ββ decay process. This apparatus consists of an up-to 6 Tesla, open-access spectroscopy ion-trap, surrounded radially by up to 7 planar Si(Li) detectors which are separated from the trap by thin Be windows. This configuration provides a significant increase in sensitivity for the detection of low-energy photons by providing backing-free ion storage and eliminating charged-particle-induced backgrounds. An intense electron beam is also employed to increase the charge-states of the trapped ions, thus providing storage times on the order of minutes, allowing for decay-spectroscopy measurements. The technique of multiple ion-bunch stacking was also recently demonstrated, which further extends the measurement possibilities of this apparatus. The current status of the facility and initial results from a 116In measurement are presented.

  12. Low background screening capability in the UK

    NASA Astrophysics Data System (ADS)

    Ghag, Chamkaur

    2015-08-01

    Low background rare event searches in underground laboratories seeking observation of direct dark matter interactions or neutrino-less double beta decay have the potential to profoundly advance our understanding of the physical universe. Successful results from these experiments depend critically on construction from extremely radiologically clean materials and accurate knowledge of subsequent low levels of expected background. The experiments must conduct comprehensive screening campaigns to reduce radioactivity from detector components, and these measurements also inform detailed characterisation and quantification of background sources and their impact, necessary to assign statistical significance to any potential discovery. To provide requisite sensitivity for material screening and characterisation in the UK to support our rare event search activities, we have re-developed our infrastructure to add ultra-low background capability across a range of complementary techniques that collectively allow complete radioactivity measurements. Ultra-low background HPGe and BEGe detectors have been installed at the Boulby Underground Laboratory, itself undergoing substantial facility re-furbishment, to provide high sensitivity gamma spectroscopy in particular for measuring the uranium and thorium decay series products. Dedicated low-activity mass spectrometry instrumentation has been developed at UCL for part per trillion level contaminant identification to complement underground screening with direct U and Th measurements, and meet throughput demands. Finally, radon emanation screening at UCL measures radon background inaccessible to gamma or mass spectrometry techniques. With this new capability the UK is delivering half of the radioactivity screening for the LZ dark matter search experiment.

  13. Low background screening capability in the UK

    SciTech Connect

    Ghag, Chamkaur

    2015-08-17

    Low background rare event searches in underground laboratories seeking observation of direct dark matter interactions or neutrino-less double beta decay have the potential to profoundly advance our understanding of the physical universe. Successful results from these experiments depend critically on construction from extremely radiologically clean materials and accurate knowledge of subsequent low levels of expected background. The experiments must conduct comprehensive screening campaigns to reduce radioactivity from detector components, and these measurements also inform detailed characterisation and quantification of background sources and their impact, necessary to assign statistical significance to any potential discovery. To provide requisite sensitivity for material screening and characterisation in the UK to support our rare event search activities, we have re-developed our infrastructure to add ultra-low background capability across a range of complementary techniques that collectively allow complete radioactivity measurements. Ultra-low background HPGe and BEGe detectors have been installed at the Boulby Underground Laboratory, itself undergoing substantial facility re-furbishment, to provide high sensitivity gamma spectroscopy in particular for measuring the uranium and thorium decay series products. Dedicated low-activity mass spectrometry instrumentation has been developed at UCL for part per trillion level contaminant identification to complement underground screening with direct U and Th measurements, and meet throughput demands. Finally, radon emanation screening at UCL measures radon background inaccessible to gamma or mass spectrometry techniques. With this new capability the UK is delivering half of the radioactivity screening for the LZ dark matter search experiment.

  14. Total internal reflection fluorescence correlation spectroscopy (TIR-FCS) with low background and high count-rate per molecule

    NASA Astrophysics Data System (ADS)

    Hassler, Kai; Leutenegger, Marcel; Rigler, Per; Rao, Ramachandra; Rigler, Rudolf; Gösch, Michael; Lasser, Theo

    2005-09-01

    We designed a fluorescence correlation spectroscopy (FCS) system for measurements on surfaces. The system consists of an objective-type total internal reflection fluorescence (TIRF) microscopy setup, adapted to measure FCS. Here, the fluorescence exciting evanescent wave is generated by epi-illumination through the periphery of a high NA oil-immersion objective. The main advantages with respect to conventional FCS systems are an improvement in terms of counts per molecule (cpm) and a high signal to background ratio. This is demonstrated by investigating diffusion as well as binding and release of single molecules on a glass surface. Furthermore, the size and shape of the molecule detection efficiency (MDE) function was calculated, using a wave-vectorial approach and taking into account the influence of the dielectric interface on the emission properties of fluorophores.

  15. Simultaneous beta and gamma spectroscopy

    DOEpatents

    Farsoni, Abdollah T.; Hamby, David M.

    2010-03-23

    A phoswich radiation detector for simultaneous spectroscopy of beta rays and gamma rays includes three scintillators with different decay time characteristics. Two of the three scintillators are used for beta detection and the third scintillator is used for gamma detection. A pulse induced by an interaction of radiation with the detector is digitally analyzed to classify the type of event as beta, gamma, or unknown. A pulse is classified as a beta event if the pulse originated from just the first scintillator alone or from just the first and the second scintillator. A pulse from just the third scintillator is recorded as gamma event. Other pulses are rejected as unknown events.

  16. The LBNL Low Background Facility - Services and Recent Updates

    NASA Astrophysics Data System (ADS)

    Thomas, Keenan; Smith, Alan; Norman, Eric; Chan, Yuen-Dat; Poon, Alan; Lesko, Kevin

    2014-09-01

    The Low Background Facility (LBF) at Lawrence Berkeley National Laboratory (LBNL) in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background laboratory on the surface at LBNL and at a recently established underground location (4300 m.w.e) at the Sanford Underground Research Facility (SURF) in Lead, SD (relocated from Oroville, CA). These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K) or common cosmogenic/anthropogenic products; active screening via neutron activation analysis for U,Th, and K as well as a variety of stable isotopes; and neutron flux/beam characterization through the use of monitors. A general overview of the facilities, services, and sensitivities will be presented. Recent activities and upgrades will also be described in detail including an overview of the recently installed counting system at SURF. The LBF is open to any users for counting services or collaboration on a wide variety of experiments and projects. The Low Background Facility (LBF) at Lawrence Berkeley National Laboratory (LBNL) in Berkeley, California provides low background gamma spectroscopy services to a wide array of experiments and projects. The analysis of samples takes place within two unique facilities; locally within a carefully-constructed, low background laboratory on the surface at LBNL and at a recently established underground location (4300 m.w.e) at the Sanford Underground Research Facility (SURF) in Lead, SD (relocated from Oroville, CA). These facilities provide a variety of gamma spectroscopy services to low background experiments primarily in the form of passive material screening for primordial radioisotopes (U, Th, K) or common cosmogenic

  17. Planetary gamma-ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Reedy, R. C.

    1978-01-01

    The measured intensities of certain gamma rays of specific energies escaping from a planetary surface can be used to determine the abundances of a number of elements. The fluxes of the more intense gamma-ray lines emitted from 32 elements were calculated using current nuclear data and existing models for the source processes. The source strengths for neutron-capture reactions were modified from those previously used. The fluxes emitted form a surface of average lunar composition are reported for 292 gamma-ray lines. These theoretical fluxes were used elsewhere to convert the data from the Apollo gamma-ray spectrometers to elemental abundances and can be used with measurements from future missions to map the concentrations of a number of elements over a planet's surface. Detection sensitivities for these elements are examined and applications of gamma-ray spectroscopy for future orbiters to Mars and other solar-system objects are discussed.

  18. Ultra high vacuum high precision low background setup with temperature control for thermal desorption mass spectroscopy (TDA-MS) of hydrogen in metals.

    PubMed

    Merzlikin, Sergiy V; Borodin, S; Vogel, D; Rohwerder, M

    2015-05-01

    In this work, a newly developed UHV-based high precision low background setup for hydrogen thermal desorption analysis (TDA) of metallic samples is presented. Using an infrared heating with a low thermal capacity enables a precise control of the temperature and rapid cool down of the measurement chamber. This novel TDA-set up is superior in sensitivity to almost every standard hydrogen analyzer available commercially due to the special design of the measurement chamber, resulting in a very low hydrogen background. No effects of background drift characteristic as for carrier gas based TDA instruments were observed, ensuring linearity and reproducibility of the analysis. This setup will prove to be valuable for detailed investigations of hydrogen trapping sites in steels and other alloys. With a determined limit of detection of 5.9×10(-3)µg g(-1) hydrogen the developed instrument is able to determine extremely low hydrogen amounts even at very low hydrogen desorption rates. This work clearly demonstrates the great potential of ultra-high vacuum thermal desorption mass spectroscopy instrumentation. PMID:25702992

  19. Gamma ray spectroscopy in astrophysics. [conferences

    NASA Technical Reports Server (NTRS)

    Cline, T. L. (Editor); Ramaty, R. (Editor)

    1978-01-01

    Experimental and theoretical aspects of gamma ray spectroscopy in high energy astrophysics are discussed. Line spectra from solar, stellar, planetary, and cosmic gamma rays are examined as well as HEAO investigations, the prospects of a gamma ray observatory, and follow-on X-ray experiments in space.

  20. Gamma spectroscopy of environmental samples

    NASA Astrophysics Data System (ADS)

    Siegel, P. B.

    2013-05-01

    We describe experiments for the undergraduate laboratory that use a high-resolution gamma detector to measure radiation in environmental samples. The experiments are designed to instruct the students in the quantitative analysis of gamma spectra and secular equilibrium. Experiments include the radioactive dating of Brazil nuts, determining radioisotope concentrations in natural samples, and measurement of the 235U abundance in uranium rich rocks.

  1. Astrophysical gamma-ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Ramaty, R.; Lingenfelter, R. E.; Kozlovsky, B.

    1979-01-01

    Observations of gamma-ray lines from solar flares, the Galactic Center, and transient celestial events are reviewed. The lines observed in each case are identified, and possible emission sources are considered. Future prospects for gamma-ray line astronomy are briefly discussed.

  2. Simultaneous beta/gamma digital spectroscopy

    NASA Astrophysics Data System (ADS)

    Farsoni, Abdollah T.

    A state-of-the-art radiation detection system for simultaneous spectroscopy of beta-particles and gamma-rays has been developed. The system utilizes a triple-layer phoswich detector and a customized Digital Pulse Processor (DPP) built in our laboratory. The DPP board was designed to digitally capture the analog signal pulses and, following several digital preprocessing steps, transfer valid pulses to the host computer for further digital processing. A MATLAB algorithm was developed to digitally discriminate beta and gamma events and reconstruct separate beta and gamma-ray energy spectra with minimum crosstalk. The spectrometer proved to be an effective tool for recording separate beta and gamma-ray spectra from mixed radiation fields. The system as a beta-gamma spectrometer will have broad-ranging applications in nuclear non-proliferation, radioactive waste management, worker safety, systems reliability, dose assessment, and risk analysis.

  3. Low Background Micromegas in CAST

    NASA Astrophysics Data System (ADS)

    Garza, J. G.; Aune, S.; Aznar, F.; Calvet, D.; Castel, J. F.; Christensen, F. E.; Dafni, T.; Davenport, M.; Decker, T.; Ferrer-Ribas, E.; Galán, J.; García, J. A.; Giomataris, I.; Hill, R. M.; Iguaz, F. J.; Irastorza, I. G.; Jakobsen, A. C.; Jourde, D.; Mirallas, H.; Ortega, I.; Papaevangelou, T.; Pivovaroff, M. J.; Ruz, J.; Tomás, A.; Vafeiadis, T.; Vogel, J. K.

    2015-11-01

    Solar axions could be converted into x-rays inside the strong magnetic field of an axion helioscope, triggering the detection of this elusive particle. Low background x-ray detectors are an essential component for the sensitivity of these searches. We report on the latest developments of the Micromegas detectors for the CERN Axion Solar Telescope (CAST), including technological pathfinder activities for the future International Axion Observatory (IAXO). The use of low background techniques and the application of discrimination algorithms based on the high granularity of the readout have led to background levels below 10-6 counts/keV/cm2/s, more than a factor 100 lower than the first generation of Micromegas detectors. The best levels achieved at the Canfranc Underground Laboratory (LSC) are as low as 10-7 counts/keV/cm2/s, showing good prospects for the application of this technology in IAXO. The current background model, based on underground and surface measurements, is presented, as well as the strategies to further reduce the background level. Finally, we will describe the R&D paths to achieve sub-keV energy thresholds, which could broaden the physics case of axion helioscopes.

  4. Gamma-ray spectroscopy - Status and prospects

    NASA Technical Reports Server (NTRS)

    Matteson, J. L.

    1983-01-01

    Contemporary gamma-ray spectroscopy instruments and their results are reviewed. Sensitivities of 10 to the -4th to 10 to the -3rd ph/sq cm-sec have been achieved for steady sources and 10 to the -2nd to 1 ph/sq cm-sec for transient sources. This has led to the detection of gamma-ray lines from more than 40 objects representing 6 classes of astrophysical phenomena. The lines carry model-independent information and are of fundamental importance to theoretical modeling and our understanding of the objects. The objectives and anticipated results of future instruments are discussed. Several instruments in development will have a factor of 10 sensitivity improvement to certain phenomena over contemporary instruments. A factor of 100 improvement in sensitivity will allow the full potential of gamma-ray spectroscopy to be realized. Instrument concepts which would achieve this with both present and advanced techniques are discussed.

  5. Low Background Counting At SNOLAB

    SciTech Connect

    Lawson, Ian; Cleveland, Bruce

    2011-04-27

    It is a continuous and ongoing effort to maintain radioactivity in materials and in the environment surrounding most underground experiments at very low levels. These low levels are required so that experiments can achieve the required detection sensitivities for the detection of low-energy neutrinos, searches for dark matter and neutrinoless double-beta decay. SNOLAB has several facilities which are used to determine these low background levels in the materials and the underground environment. This proceedings will describe the SNOLAB High Purity Germanium Detector which has been in continuous use for the past five years and give results of many of the items that have been counted over that period. Brief descriptions of SNOLAB's alpha-beta and electrostatic counters will be given, and the radon levels at SNOLAB will be discussed.

  6. Gamma-ray spectroscopy - Requirements and prospects

    NASA Technical Reports Server (NTRS)

    Matteson, James L.

    1991-01-01

    The only previous space instrument which had sufficient spectral resolution and directionality for the resolution of astrophysical sources was the Gamma-Ray Spectrometer carried by HEAO-3. A broad variety of astrophysical investigations entail gamma-ray spectroscopy of E/Delta-E resolving power of the order of 500 at 1 MeV; it is presently argued that a sensitivity to narrow gamma-ray lines of a few millionths ph/sq cm, from about 10 keV to about 10 MeV, should typify the gamma-ray spectrometers of prospective missions. This performance is achievable with technology currently under development, and could be applied to the NASA's planned Nuclear Astrophysics Explorer.

  7. Low-Background Counting at Homestake

    NASA Astrophysics Data System (ADS)

    Marshall, Iseley

    2009-10-01

    Background characterization at Homestake is an ongoing project crucial to the experiments located there. From neutrino physics to WIMP detection, low-background materials and their screening require highly sensitive detectors. Naturally, shielding is needed to lower ``noise'' in these detectors. Because of its vast depth, Homestake will be effective in shielding against cosmic-ray radiation. This means little, however, if radiation from materials used still interferes. Specifically, our group is working on designing the first low-background counting facility at the Homestake mine. Using a high-purity germanium crystal detector from ORTEC, measurements will be taken within a shield that is made to specifically account for radiation underground and fits the detector. Currently, in the design, there is a layer of copper surrounded by an intricate stainless steel casing, which will be manufactured air tight to accommodate for nitrogen purging. Lead will surround the stainless steel shell to further absorb gamma rays. A mobile lift system has been designed for easy access to the detector. In the future, this project will include multiple testing stations located in the famous Davis Cavern where future experiments will have the ability to use the site as an efficient and accurate counting facility for their needs (such as measuring radioactive isotopes in materials). Overall, this detector (and its shield system) is the beginning of a central testing facility that will serve Homestake's scientific community.

  8. The Berkeley Low Background Facility and the Black Hills State University Underground Campus at SURF

    NASA Astrophysics Data System (ADS)

    Thomas, Keenan; Mount, Brianna; Lesko, Kevin; Norman, Eric; Smith, Alan; Poon, Alan; Chan, Yuen-Dat

    2015-10-01

    The Berkeley Low Background Facility at LBNL provides a variety of low background gamma spectroscopy services to a variety of projects and experiments. It operates HPGe spectrometers in two unique facilities: a surface low background lab at LBNL and underground (4300 m.w.e.) at the Sanford Underground Research Facility in Lead, SD. A large component of the measurements performed by the BLBF are for ultralow background experiments concerned with U, Th, K, and other radioisotopes within candidate construction materials to be used to construct sensitive detectors, such as those studying dark matter or neutrinos. The BLBF also makes a variety of environmental measurements in search of other radioisotopes, such as fallout from the Fukushima nuclear power plant accident in 2011 and other radioisotope monitoring activities. A general overview of the services and facilities will be presented. In 2015, the BLBF will be relocating its underground counting stations to a new, dedicated space on the 4850L of SURF. The Black Hills State University Underground Campus will host several low background counting stations and operate in a coordinated manner to provide low background measurements to the scientific community. An overview and description of the BHUC will be presented.

  9. Low background aspects of GERDA

    SciTech Connect

    Simgen, Hardy

    2011-04-27

    The GERDA experiment operates bare Germanium diodes enriched in {sup 76}Ge in an environment of pure liquid argon to search for neutrinoless double beta decay. A very low radioactive background is essential for the success of the experiment. We present here the research done in order to remove radio-impurities coming from the liquid argon, the stainless steel cryostat and the front-end electronics. We found that liquid argon can be purified efficiently from {sup 222}Rn. The main source of {sup 222}Rn in GERDA is the cryostat which emanates about 55 mBq. A thin copper shroud in the center of the cryostat was implemented to prevent radon from approaching the diodes. Gamma ray screening of radio-pure components for front-end electronics resulted in the development of a pre-amplifier with a total activity of less than 1 mBq {sup 228}Th.

  10. Quantification of 235U and 238U activity concentrations for undeclared nuclear materials by a digital gamma-gamma coincidence spectroscopy.

    PubMed

    Zhang, Weihua; Yi, Jing; Mekarski, Pawel; Ungar, Kurt; Hauck, Barry; Kramer, Gary H

    2011-06-01

    The purpose of this study is to investigate the possibility of verifying depleted uranium (DU), natural uranium (NU), low enriched uranium (LEU) and high enriched uranium (HEU) by a developed digital gamma-gamma coincidence spectroscopy. The spectroscopy consists of two NaI(Tl) scintillators and XIA LLC Digital Gamma Finder (DGF)/Pixie-4 software and card package. The results demonstrate that the spectroscopy provides an effective method of (235)U and (238)U quantification based on the count rate of their gamma-gamma coincidence counting signatures. The main advantages of this approach over the conventional gamma spectrometry include the facts of low background continuum near coincident signatures of (235)U and (238)U, less interference from other radionuclides by the gamma-gamma coincidence counting, and region-of-interest (ROI) imagine analysis for uranium enrichment determination. Compared to conventional gamma spectrometry, the method offers additional advantage of requiring minimal calibrations for (235)U and (238)U quantification at different sample geometries. PMID:21411329

  11. Optimized Derivative Kernels for Gamma Ray Spectroscopy

    SciTech Connect

    Vlachos, D. S.; Kosmas, O. T.; Simos, T. E.

    2007-12-26

    In gamma ray spectroscopy, the photon detectors measure the number of photons with energy that lies in an interval which is called a channel. This accumulation of counts produce a measuring function that its deviation from the ideal one may produce high noise in the unfolded spectrum. In order to deal with this problem, the ideal accumulation function is interpolated with the use of special designed derivative kernels. Simulation results are presented which show that this approach is very effective even in spectra with low statistics.

  12. Directions in gamma-ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Gehrels, Neil; Candey, Robert M.

    1990-01-01

    Current and future instrumentation for gamma-ray spectroscopy in the spectral range from 10 keV to 10 MeV is described. New technologies for Germanium (Ge) spectrometers and emerging detector technologies are highlighted. Scientific objectives are considered, with emphasis on capabilities beyond those of the Nuclear Astrophysics Explorer (NAE). A list of instrument requirements is given. Technologies under development for an NAE-era spectrometer are presented. Spectrometers beyond NAE and other types of future technologies are discussed, and a partial list of current and future spectrometers is provided.

  13. Microsatellite gamma-ray spectroscopy experiment

    NASA Astrophysics Data System (ADS)

    Asa, G.; Ruzin, Arie; Jakobson, Claudio G.; Shaviv, G.; Nemirovsky, Yael

    1999-10-01

    Preliminary results from Gamma ray experiment installed on a micro-satellite, Techsat 1, are reported. The experiment is based on CdZnTe detectors coupled to custom designed CMOS electronics, which includes low noise charge sensitive preamplifiers, pulse shaping amplifiers and sampling circuits. It was realized as a mile stone towards a micro- satellite mounted Gamma ray space telescope. The experiment is a stand-alone spectroscopy system that measures the radiation inside the micro-satellite and transmits the spectra to ground station via the main satellite computer. The radiation level inside micro-satellites is expected to be significantly lower compared to that inside large satellites. Additional goal of the experiment is to test the CdZnTe detectors and the front-end electronics, implemented in a standard CMOS process, under space radiation environment. In particular, the degradation in performance will be monitored. The Techsat 1 micro-satellite has been designed and constructed at Technion-Israel Institute of Technology. The satellite is approximately 50 X 50 X 50 cm-3 cube with a total weight of about 50 kilograms. It was successfully launched in July 1998 to a 820 km orbit.

  14. Validating the Melusine Gamma Spectroscopy Tool

    SciTech Connect

    Erikson, Luke E.; Keillor, Martin E.; Stavenger, Timothy J.

    2013-11-26

    This technical report describes testing to evaluate the gamma spectroscopy tool, Melusine, under development by Pacific Northwest National Laboratory. The goal was to verify that the software can successfully be used to provide accurate results and statistical uncertainties for the detection of isotopes of interest and their activities. Of special interest were spectra similar to those produced by radionuclide stations that contribute to the Comprehensive Nuclear Test Ban Treaty Organization’s International Monitoring System. Two data sets were used to test Melusine’s capabilities. The first was the result of a multi-lab calibration effort based on neutron activations produced at the University of California at Davis. The second was taken from the Proficiency Test Exercises conducted by the CTBTO directly in 2005. In 37 of 42 cases, Melusine produced results in agreement with the best answer presently available, in most cases with calculated uncertainties comparable to or better than competing analyses. In fact, Melusine technically provided one more result than CTBTO’s PTE analyses that agreed with the “book answer” (Monte Carlo simulation). Despite these promising results, the Melusine software is still under development. Effort is especially needed to simplify its analysis process, improve stability, and provide user documentation. Some significant analysis tasks require further vetting, such as those to address summing effects. However, our test results indicate that Melusine’s calculations as presently implemented are sound and can be used to reliably analyze spectra from the CTBTO’s radionuclide stations.

  15. Gamma-Ray Spectroscopy of Nearby OB Associations

    NASA Technical Reports Server (NTRS)

    Kaaret, Philip

    1997-01-01

    This final report is a summary of the study on gamma ray spectroscopy of nearby OB associations. The goal of this work is to investigate the gamma ray line emission detected with the Compton Telescope (COMPTEL) from the Orion star forming region. This is accomplished by searching for similar emission from other nearby OB associations.

  16. DUSEL Ultra-Low Background Counting Facility

    NASA Astrophysics Data System (ADS)

    Thomas, Keenan

    2007-10-01

    The Homestake Mine in western South Dakota has been confirmed by the National Science Foundation (NSF) as the site for a Deep Underground Science and Engineering Laboratory (DUSEL). Many of the physics, geosciences, and microbiology experiments in the facility will be funded by DOE and NSF, and will benefit the missions of these agencies. In support of these programs, physics faculty in South Dakota and scientists at Lawrence Berkeley National Laboratory have been working together to establish a multidisciplinary research cluster to provide baseline characterization for physics and geosciences/geomicrobiology experiments at the Homestake Mine through an Ultra-Low Background Counting Facility (ULBCoF). The proposed project utilizes two low-background germanium detectors with massive shielding underground to carefully analyze materials for low background experiments. Low background experiments such as double-beta decay, solar neutrino, geoneutrino, and dark matter must control the purity of all the materials used in the construction of a detector. Measuring such low counting rates is a very challenging task that will be best accomplished by primarily using high purity germanium (HPGe) detectors.

  17. Low background counting techniques at SNOLAB

    SciTech Connect

    Lawson, Ian; Cleveland, Bruce

    2013-08-08

    Many of the experiments currently searching for dark matter, studying properties of neutrinos or searching for neutrinoless double beta decay require very low levels of radioactive backgrounds both in their own construction materials and in the surrounding environment. These low background levels are required so that the experiments can achieve the required sensitivities for their searches. SNOLAB has several facilities which are used to directly measure these radioactive backgrounds. This proceedings will describe SNOLAB's High Purity Germanium Detectors, one of which has been in continuous use for the past seven years measuring materials for many experiments in operation or under construction at SNOLAB. A description of the characterisation of SNOLAB's new germanium well detector will be presented. In addition, brief descriptions of SNOLAB's alpha-beta and electrostatic counters will be presented and a description of SNOLAB's future low background counting laboratory will be given.

  18. Solar flare gamma-ray line spectroscopy

    NASA Technical Reports Server (NTRS)

    Murphy, R. J.; Forrest, D. J.; Ramaty, R.; Kozlovsky, B.

    1985-01-01

    The techniques and the results of solar elemental abundance determinations using observations of gamma ray lines from the April 27 1981 olar flare were outlined. The techniques are elaborated on and observed and the best-fitting theoretical spectra are presented. Numerical values for the photon fluences and the total number of protons involved in the thick-target production of these gamma rays are derived.

  19. Low-background detector arrays for infrared astronomy

    NASA Technical Reports Server (NTRS)

    Mccreight, C. R.; Estrada, J. A.; Goebel, J. H.; Mckelvey, M. E.; Mckibbin, D. D.; Mcmurray, R. E., Jr.; Weber, T. T.

    1989-01-01

    The status of a program which develops and characterizes integrated infrared (IR) detector array technology for space astronomical applications is described. The devices under development include intrinsic, extrinsic silicon, and extrinsic germanium detectors, coupled to silicon readout electronics. Low-background laboratory test results include measurements of responsivity, noise, dark current, temporal response, and the effects of gamma-radiation. In addition, successful astronomical imagery has been obtained on some arrays from this program. These two aspects of the development combine to demonstrate the strong potential for integrated array technology for IR space astronomy.

  20. HYPERNUCLEAR STRUCTURE FROM GAMMA-RAY SPECTROSCOPY.

    SciTech Connect

    MILLENER,D.J.

    2003-10-14

    The energies of p-shell hypernuclear {gamma} rays obtained from recent experiments using the Hyperball at BNL and KEK are used to constrain the YN interaction which enters into shell-model calculations which include both {Lambda} and {Sigma} configurations.

  1. A system for simultaneous beta and gamma spectroscopy

    NASA Astrophysics Data System (ADS)

    Farsoni, A. T.; Hamby, D. M.

    2007-08-01

    A state-of-the-art radiation detection system for real-time and simultaneous spectroscopy of beta-particles and gamma-rays has been developed. The system utilizes a triple-layer phoswich detector and a customized Digital Pulse Processor (DPP) designed and built in our laboratory. The DPP board digitally captures the analog signal pulses and, following several digital preprocessing steps, transfers valid pulses to the host computer for further digital processing. A resolving algorithm also was developed to digitally discriminate beta and gamma events, and reconstruct separate beta and gamma-ray energy spectra with minimal crosstalk. The spectrometer has proven to be an effective tool for recording separate beta and gamma-ray spectra from mixed radiation fields. The system as a beta-gamma spectrometer will have broad-ranging applications in nuclear non-proliferation, radioactive waste management, worker safety, systems reliability, dose assessment, and risk analysis.

  2. Nucleosynthesis and astrophysical gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Jacobson, Allan S.

    1987-01-01

    The HEAO-3 gamma ray spectrometer has provided evidence in the quest for the understanding of complex element formation in the universe with the discovery of Al-26 in the interstellar medium. It has demonstrated that the synthesis of intermediate mass nuclei is currently going on in the galaxy. This discovery was confirmed by the Solar Maximum Mission. The flux is peaked near the galactic center and indicates about 3 solar masses of Al-26 in the interstellar medium, with an implied ratio of Al-26/Al-27 = .00001. Several possible distributions were studied but the data gathered thus far do not allow discrimination between them. It is felt that only the spaceflight of a high resolution gamma ray spectrometer with adequate sensitivity will ultimately resolve the issue of the source of this material.

  3. Low background techniques applied in the BOREXINO experiment

    SciTech Connect

    Zuzel, G.

    2015-08-17

    The BOREXINO detector, located in the Gran Sasso National Laboratory in Italy, has been designed for real-time spectroscopy of low-energy solar neutrinos. Within the experiment several novel background reduction and assay techniques have been established. In many cases they are still the most sensitive world-wide. Developed methods and apparatus provided tools for a strict quality control program during the construction phase of the BOREXINO detector, which was the key to meet the background requirements. Achievement of extremely low background rate opened the possibility to probe in realtime almost entire spectrum of the solar neutrinos.

  4. Low Background Assay Results for LZ

    NASA Astrophysics Data System (ADS)

    Oliver-Mallory, Kelsey; Thomas, Keenan; Lux-Zeplin Collaboration; Berkeley Low Background Facility Team

    2016-03-01

    The next generation dark matter experiment LUX-ZEPLIN (LZ) requires careful control of intrinsic radioactivity in all critical detector components in order to reach its unprecedented target sensitivity to Weakly Interacting Massive Particles (WIMPs): 2 ×10-48 cm2 at 50 GeV/c2. Appropriate material selection is essential to meeting this goal, and an extensive campaign of low background screening is currently being carried out using assay devices at the Sanford Underground Research Facility and the Boulby Underground Laboratory. We will present results from this work, including measurements for the Ti cryostat, PMT bases, PMT raw materials, PTFE, and other components. This work was partially supported by the U.S. Department of Energy (DOE) under Award Number DE-AC02-05CH11231, and is based upon work supported by the National Science Foundation Graduate Research Fellowship under Grant No. 1106400.

  5. Image Recognition Techniques for Gamma Spectroscopy

    SciTech Connect

    Vlachos, D. S.; Tsabaris, C. G.

    2007-12-26

    Photons, after generated from a radioactive source and before they deposit their energy in a photo detector, are subsequent to multiple scattering mechanisms. As a result, the measured energy from the photo detector is different from the energy the photon had when generated. This is known as folding of the photon energy. Moreover, statistical fluctuation inside the detector contribute to energy folding. In this work, a new method is presented for unfolding the gamma ray spectrum. The method uses a 2-dimensional representation of the measured spectrum (image) and then uses image recognition techniques, and especially differential edge detection, to generate the original spectrum.

  6. Solar abundances from gamma-ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Ramaty, R.

    1989-01-01

    Determinations of solar abundances from gamma-ray line observations are reviewed. The principal results are: (1) in flare loops, at atmospheric heights betwen the transition region and the upper photosphere, the Mg/O ratio is higher by about a factor of 3 than in the photosphere, while the C/O ratio is essentially photospheric; (2) in the same region, the Ne/O ratio is higher by about a factor of 3 than the Ne/O ratio in the corona; (3) the photospheric He-3/H ratio is less than 0.000035. These results, combined with other data, suggest abundance variations in the solar atmosphere, possibly resulting from charge and mass dependent transport.

  7. Gamma-ray spectroscopy of hypernuclei

    SciTech Connect

    Chrien, R.E.

    1984-01-01

    The study of hypernuclei is a frontier area of nuclear physics. As more intense beams of strange mesons have become available, methods of in-beam spectroscopy have been applied to the study of hypernuclei. The feasibility of detecting hypernuclear electromagnetic radiation has been demonstrated at the Brookhaven Alternating Gradient Synchrotron. Studies have been made of the effective LAMBDA hyperon-nucleon interaction in p-shell hypernuclei. The first results are described and they place useful constraints on the effective interaction and the shell model description of hypernuclear states.

  8. Combined Gamma Ray/neutron Spectroscopy for Mapping Lunar Resources

    NASA Technical Reports Server (NTRS)

    Reedy, R. C.; Byrd, R. C.; Drake, D. M.; Feldman, W. C.; Masarik, J.; Moss, C. E.

    1992-01-01

    Some elements in the Moon can be resources, such as hydrogen and oxygen. Other elements, like Ti or the minerals in which they occur, such as ilmenite, could be used in processing lunar materials. Certain elements can also be used as tracers for other elements or lunar processes, such as hydrogen for mature regoliths with other solar-wind-implanted elements like helium, carbon, and nitrogen. A complete knowledge of the elemental composition of a lunar region is desirable both in identifying lunar resources and in lunar geochemical studies, which also helps in identifying and using lunar resources. The use of gamma ray and neutron spectroscopy together to determine abundances of many elements in the top few tens of centimeters of the lunar surface is discussed. To date, very few discussions of elemental mapping of planetary surfaces considered measurements of both gamma rays and the full range of neutron energies. The theories for gamma ray and neutron spectroscopy of the Moon and calculations of leakage fluxes are presented here with emphasis on why combined gamma ray/neutron spectroscopy is much more powerful than measuring either radiation alone.

  9. Slănic-Prahova low background calibration facility.

    PubMed

    Celarel, Aurelia; Duliu, O G; Bercea, S; Cenusa, C

    2016-03-01

    The reduced background of 2 nSv h(-1) of the Slănic-Prahova Low Background Radiation Laboratory allowed installing a calibration stand for low-dose-rates dosimetry. The stand is provided with (60)Co, (137)Cs and (241)Am low activity sources. A Physikalisch-Technische Bundesanstalt-calibrated AUTOMESS 6150 AD-6 dose rate meter with a 6150 AD-b/H external probe was used to check to what extent this stand could serve as a low background calibration facility. A detailed analysis of possible uncertainties in measuring dose rates evidenced an extended uncertainty related to the certified calibration as well as instrument readings of about 3 % for a confidence level of 95 %. In these conditions, the experimentally determined dose rates for all three gamma ray sources and for source-to-probe distances varying between 0.3 and 2.0 m confirmed a good correlation between the calculated and measured dose rates. At the same time, dose rates perfectly obey to an inverse squared distances law. PMID:26001826

  10. Delayed Gamma-Ray Spectroscopy for Spent Nuclear Fuel Assay

    SciTech Connect

    Campbell, Luke W.; Hunt, Alan W.; Ludewigt, Bernhard A.; Mozin, Vladimir V.

    2012-04-01

    High-energy, beta-delayed gamma-ray spectroscopy is investigated as a non-destructive assay technique for the determination of plutonium mass in spent nuclear fuel. This approach exploits the unique isotope-specific signatures contained in the delayed gamma-ray emission spectra detected following active interrogation with an external neutron source. A high fidelity modeling approach is described that couples radiation transport, analytical decay/depletion, and a newly developed gamma-ray emission source reconstruction code. Initially simulated and analyzed was a “one-pass” delayed gamma-ray assay that focused on the long-lived signatures. Also presented are the results of an independent study that investigated “pulsed mode” measurements, to capture the more isotope-specific, short-lived signatures. Initial modeling results outlined in this paper suggest that delayed gamma-ray assay of spent nuclear fuel assemblies can be accomplished with a neutron generator of sufficient strength and currently available gamma-ray detectors.

  11. Labr3:Ce scintillators for gamma ray spectroscopy

    SciTech Connect

    Shah, K.S.; Glodo, J.; Klugerman, M.; Moses, W.W.; Derenzo, S.E.; Weber, M.J.

    2002-12-02

    In this paper, we report on a relatively new scintillator -LaBr3 for gamma ray spectroscopy. Crystals of this scintillator have beengrown using Bridgman process. This material when doped with cerium hashigh light output (~;60,000 photons/MeV) and fast principal decayconstant (less than 25 ns). Furthermore, it shows excellent energyresolution for gamma-ray detection. Energy resolution of 3.2 percent(FWHM) has been achieved for 662 keV photons (137Cs source) at roomtemperature. High timing resolution (260 ps - FWHM) has been recordedwith LaBr3-PMT and BaF2-PMT detectors operating in coincidence mode using511 keV positron annihilation gamma-ray pairs. Details of itsscintillation properties, and variation of these properties with changingcerium concentration are reported. Potential applications of thismaterial are also addressed.

  12. High resolution gamma-ray spectroscopy at GANIL

    SciTech Connect

    France, G. de

    2014-11-11

    Gamma-ray spectroscopy is intensively used at GANIL to measure low lying states in exotic nuclei on the neutron-rich as well as on the neutron-deficient side of the nuclear chart. On the neutron deficient border, gamma-rays have been observed for the first time in {sup 92}Pd. The level scheme which could be established points to the role of isoscalar pairing. On the neutron rich side, the lifetime of excited states in nuclei around {sup 68}Ni have been been measured using the plunger technique. This allows us to study the evolution of collectivity in a broad range of nuclei. In 2014 GANIL will host the AGATA array for a campaign of at least 2 years. This array is based on the gamma-ray tracking technique, which allows an impressive gain in resolving power.

  13. A pneumatic sample changer for gamma-ray spectroscopy

    USGS Publications Warehouse

    Massoni, C.J.; Fones, R.V.; Simon, F.O.

    1973-01-01

    A gravity-feed, pneumatic-ejection sample changer has been developed. The changer is suitable for both flat and well-type detectors and permits the continuous use of gamma-ray spectroscopy equipment 24 h a day, 7 days a week. The electronic circuitry has a fail-safe feature which stops the operation of the changer if a malfunction occurs. ?? 1973 The American Institute of Physics.

  14. BATSE spectroscopy catalog of bright gamma-ray bursts

    NASA Technical Reports Server (NTRS)

    Schaefer, Bradley E.; Teegarden, Bonnard J.; Fantasia, Stephan F.; Palmer, David; Cline, Thomas L.; Matteson, James L.; Band, David L.; Ford, Lyle A.; Fishman, Gerald J.; Meegar, Charles A.

    1994-01-01

    This paper presents comprehensive results on the spectra of 30 bright gamma ray bursts (GRBs) as observed by the Spectroscopy Detectors (SDs) of the Burst And Transient Source Experiment (BATSE). The data selection was strict in including only spectra that are of high reliability for continuum shape studies. This BATSE Spectroscopy Catalog presents fluences, model fits (for five spectral models for three energy ranges), and photon spectra in a standard manner for each burst. Complete information is provided to describe the data selection and analysis procedures. The catalog results are also presented in electronic format (from the Compton Observatory Science Support Center) and CD-ROM format (AAS CD-ROM series, Vol. 2). These electronic formats also present the count spectra and detector response matrices so as to allow for independent study and fitting by researchers outside the BATSE Team. This BATSE Spectroscopy Catalog complements the catalog from BATSE Large Area Detector (LAD) data by Fishman et al. (1994).

  15. Miniaturization in x ray and gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Iwanczyk, Jan S.; Wang, Yuzhong J.; Bradley, James G.

    1993-01-01

    The paper presents advances in two new sensor technologies and a miniaturized associated electronics technology which, when combined, can allow for very significant miniaturization and for the reduction of weight and power consumption in x-ray and gamma-ray spectroscopy systems: (1) Mercuric iodide (HgI2) x-ray technology, which allows for the first time the construction of truly portable, high-energy resolution, non-cryogenic x-ray fluorescence (XRF) elemental analyzer systems, with parameters approaching those of laboratory quality cryogenic instruments; (2) the silicon avalanche photodiode (APD), which is a solid-state light sensitive device with internal amplification, capable of uniquely replacing the vacuum photomultiplier tube in scintillation gamma-ray spectrometer applications, and offering substantial improvements in size, ruggedness, low power operation and energy resolution; and (3) miniaturized (hybridized) low noise, low power amplification and processing electronics, which take full advantage of the favorable properties of these new sensors and allow for the design and fabrication of advanced, highly miniaturized x-ray and gamma-ray spectroscopy systems. The paper also presents experimental results and examples of spectrometric systems currently under construction. The directions for future developments are discussed.

  16. CdZnTe gamma ray spectrometer for orbital gamma ray spectroscopy.

    SciTech Connect

    Prettyman, T. H.; Feldman, W. C.; Fuller, K. R.; Storms, S. A.; Soldner, S. A.; Lawrence, David J. ,; Browne, M. C.; Moss, C. E.

    2001-01-01

    We present the design and analysis of a new gamma ray spectrometer for planetary science that uses an array of CdZnTe detectors to achieve the detection efficiency needed for orbital measurements. The use of CdZnTe will provide significantly improved pulse height resolution relative to scintillation-based detectors, with commensurate improvement in the accuracy of elemental abundances determined by gamma ray and neutron spectroscopy. The spectrometer can be flown either on the instrument deck of the spacecraft or on a boom. For deck-mounted systems, a BGO anticoincidence shield is included in the design to suppress the response of the CdZnTe detector to gamma rays that originate in the spacecraft. The BGO shield also serves as a backup spectrometer, providing heritage from earlier planetary science missions and reducing the risk associated with the implementation of new technology.

  17. Atmospheric measurements at Mars via gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Metzger, Albert E.; Haines, Eldon L.

    1990-01-01

    This paper describes three methods for measuring the Martian atmosphere using gamma ray spectroscopy. One method determines atmospheric thickness based on the energy-dependent differential attenuation of gamma-ray line pairs from a common element. Another makes a direct determination based on measurements of the line flux generated in the atmosphere, requires knowledge of the concentration of the component being used. The third, which makes use of a single line emitted from the surface where its flux can be established. The effects of stratigraphy on the differential attenuation method are studied, and calculations are reported which show that the measurement of atmospheric argon will be a sensitive indicator of the atmospheric fractionation accompanying CO2 precipitation in south polar regions.

  18. Elastic properties of gamma-Pu by resonant ultrasound spectroscopy

    SciTech Connect

    Migliori, Albert; Betts, J; Trugman, A; Mielke, C H; Mitchell, J N; Ramos, M; Stroe, I

    2009-01-01

    Despite intense experimental and theoretical work on Pu, there is still little understanding of the strange properties of this metal. We used resonant ultrasound spectroscopy method to investigate the elastic properties of pure polycrystalline Pu at high temperatures. Shear and longitudinal elastic moduli of the {gamma}-phase of Pu were determined simultaneously and the bulk modulus was computed from them. A smooth linear and large decrease of all elastic moduli with increasing temperature was observed. We calculated the Poisson ratio and found that it increases from 0.242 at 519K to 0.252 at 571K.

  19. Nuclear Gamma-Ray Spectroscopy at the Limit of Particle Spectroscopy

    SciTech Connect

    Dr. Norbert Pietralla

    2006-03-29

    The research project ''Nuclear Gamma-Ray Spectroscopy at the Limit of Particle Stability'' with sponsor ID ''DE-FG02-04ER41334'' started late-summer 2004 and aims at the investigation of highly excited low-spin states of selected key-nuclei in the vicinity of the particle separation threshold by means of high-resolution gamma-ray spectroscopy in electromagnetic excitation reactions. This work addresses nuclear structures with excitation energies close to the binding energy or highly excited off-yrast states in accordance with the NSAC milestones. In 2005 the program was extended towards additional use of virtual photons and theoretical description of the low-lying collective excitations in the well deformed nuclei.

  20. Purification of cerium, neodymium and gadolinium for low background experiments

    NASA Astrophysics Data System (ADS)

    Boiko, R. S.; Barabash, A. S.; Belli, P.; Bernabei, R.; Cappella, F.; Cerulli, R.; Danevich, F. A.; Incicchitti, A.; Laubenstein, M.; Mokina, V. M.; Nisi, S.; Poda, D. V.; Polischuk, O. G.; Tretyak, V. I.

    2014-01-01

    Cerium, neodymium and gadolinium contain double beta active isotopes. The most interesting are 150Nd and 160Gd (promising for 0ν2β search), 136Ce (2β+ candidate with one of the highest Q2β). The main problem of compounds containing lanthanide elements is their high radioactive contamination by uranium, radium, actinium and thorium. The new generation 2β experiments require development of methods for a deep purification of lanthanides from the radioactive elements. A combination of physical and chemical methods was applied to purify cerium, neodymium and gadolinium. Liquid-liquid extraction technique was used to remove traces of Th and U from neodymium, gadolinium and for purification of cerium from Th, U, Ra and K. Co-precipitation and recrystallization methods were utilized for further reduction of the impurities. The radioactive contamination of the samples before and after the purification was tested by using ultra-low-background HPGe gamma spectrometry. As a result of the purification procedure the radioactive contamination of gadolinium oxide (a similar purification efficiency was reached also with cerium and neodymium oxides) was decreased from 0.12 Bq/kg to 0.007 Bq/kg in 228Th, from 0.04 Bq/kg to <0.006 Bq/kg in 226Ra, and from 0.9 Bq/kg to 0.04 Bq/kg in 40K. The purification methods are much less efficient for chemically very similar radioactive elements like actinium, lanthanum and lutetium.

  1. Shielding concepts for low-background proportional counter arrays in surface laboratories.

    PubMed

    Aalseth, C E; Humble, P H; Mace, E K; Orrell, J L; Seifert, A; Williams, R M

    2016-02-01

    Development of ultra low background gas proportional counters has made the contribution from naturally occurring radioactive isotopes - primarily α and β activity in the uranium and thorium decay chains - inconsequential to instrumental sensitivity levels when measurements are performed in above ground surface laboratories. Simple lead shielding is enough to mitigate against gamma rays as gas proportional counters are already relatively insensitive to naturally occurring gamma radiation. The dominant background in these surface laboratory measurements using ultra low background gas proportional counters is due to cosmic ray generated muons, neutrons, and protons. Studies of measurements with ultra low background gas proportional counters in surface and underground laboratories as well as radiation transport Monte Carlo simulations suggest a preferred conceptual design to achieve the highest possible sensitivity from an array of low background gas proportional counters when operated in a surface laboratory. The basis for a low background gas proportional counter array and the preferred shielding configuration is reported, especially in relation to measurements of radioactive gases having low energy decays such as (37)Ar. PMID:26720259

  2. Gamma ray spectroscopy and timing using LSO and PIN photodiodes

    SciTech Connect

    Moses, W.W.; Derenzo, S.E.; Melcher, C.L.; Manente, R.A.

    1994-11-01

    The high density, high light output, and short decay time of LSO (lutetium orthosilicate, Lu{sub 2}SiO{sub 5}:Ce) make it an attractive scintillator for gamma ray spectroscopy. The low cost, small size, high quantum efficiency, and ruggedness of silicon photodiodes make them attractive photodetectors for this same application, although their high noise (Compared to a photomultiplier tube) reduces their appeal. In this work the authors measure the gamma ray energy resolution, timing accuracy, and conversion factor from gamma energy to number of electron-hole pairs produced with a 3 x 3 x 22 mm{sup 3} LSO scintillator crystal read out with a 3 x 3 mm{sup 2} silicon PIN photodiode. When the detector is excited with 511 keV photons, a photopeak centered at 1,940 e{sup {minus}} with 149 keV fwhm is observed and a timing signal with 35 ns fwhm jitter is produced. When the detector is excited with 1,275 keV photons, a photopeak centered at 4,910 e{sup {minus}} with 149 keV fwhm is observed and a timing signal with 25 ns fwhm jitter is produced. While these performance measures are inferior to those obtained with photomultiplier tubes, they are acceptable for some applications.

  3. Empirical Correction of Crosstalk in a Low-Background Germanium γ–γ Analysis System

    SciTech Connect

    Keillor, Martin E.; Erikson, Luke E.; Aalseth, Craig E.; Day, Anthony R.; Fuller, Erin S.; Glasgow, Brian D.; Hoppe, Eric W.; Hossbach, Todd W.; Mizouni, Leila K.; Myers, Allan W.; Overman, Cory T.; Seifert, Allen; Stavenger, Timothy J.

    2013-05-01

    ABSTRACT The Pacific Northwest National Laboratory is currently developing a custom software suite capable of automating many of the tasks required to accurately analyze coincident signals within gamma spectrometer arrays. During the course of this work, significant crosstalk was identified in the energy determination for spectra collected with a new low-background intrinsic germanium (HPGe) array at PNNL. The HPGe array is designed for high detection efficiency, ultra-low-background performance, and sensitive gamma gamma coincidence detection. The first half of the array, a single cryostat containing 7 HPGe crystals, was recently installed into a new shallow underground laboratory facility. This update will present a brief review of the germanium array, describe the observed crosstalk, and present a straight-forward empirical correction that significantly reduces the impact of this crosstalk on the spectroscopic performance of the system.

  4. High-spin. gamma. -ray spectroscopy: past successes, future hopes

    SciTech Connect

    Diamond, R.M.

    1983-04-01

    Nuclei can carry angular momentum by aligning individual particles along the rotation axis or by rotation of a deformed nucleus as a whole. The interweaving of these modes leads to a variety of behavior that is just beginning to be observed and explained. The discrete ..gamma..-ray studies have led to a new backbending spectroscopy, which is telling us about the details of particle alignments and monopole and quadrupole pairing. The high-spin continuum studies, as yet less well developed, are indicating changes in shape and structure, as well as particle alignments from higher shells. New developments in detector systems and in theory promise much more detailed comparisons of experiment and theory and consequent increase in our knowledge of nuclear behavior at high spin.

  5. Stopping Muons Study for Ultra-Low Background Experiments

    NASA Astrophysics Data System (ADS)

    Duncan, Daniel

    2014-09-01

    Stopping negative muons can be captured by nucleus in various materials in which neutrons and gamma rays can be produced. These energetic secondary particles can be background events for ultra-low background experiments in searching for dark matter and neutrinoless double-beta decay. The stopping negative muons captures rates in different materials have been mostly evaluated theoretically. The secondary particles in particular the energy of neutrons is not well understood for heavy elements. Experimental study of the capture rates and secondary particles is of interest of nuclear physics and rare event physics. Two plastic scintillation panels were used to create a muon detection system allowing study of stopping muons. These panels are each made of EJ200 scintillator measuring approximately 100 × 50 × 2.54 cm and attached on one side to EJ280 plastic strip measuring 2.54 × 2.54 × 50 cm. A 1'' Hamamatsu R1924A PMT is affixed to the end of each strip to collect light. The setup measures the lifetime of muons at earth's surface by detecting the time difference between stopped muons and muon decay. Data is collected for 21 hours and a mean muon lifetime of 2.02 +/- .06 microseconds is obtained. The setup will be used at Homestake to measure captures rates and secondary neutron energy spectrum. Stopping negative muons can be captured by nucleus in various materials in which neutrons and gamma rays can be produced. These energetic secondary particles can be background events for ultra-low background experiments in searching for dark matter and neutrinoless double-beta decay. The stopping negative muons captures rates in different materials have been mostly evaluated theoretically. The secondary particles in particular the energy of neutrons is not well understood for heavy elements. Experimental study of the capture rates and secondary particles is of interest of nuclear physics and rare event physics. Two plastic scintillation panels were used to create a muon

  6. Determination of plutonium isotopic composition by gamma-ray spectroscopy

    SciTech Connect

    Sampson, T.E.; Hsue, S.T.; Parker, J.L.; Johnson, S.S.; Bowersox, D.F.

    1981-01-01

    We discuss the general approach, computerized data analysis methods, and results of measurements used to determine the isotopic composition of plutonium by gamma-ray spectroscopy. The simple techniques are designed to be applicable to samples of arbitrary size, geometry, age, chemical, and isotopic composition. The combination of the gamma spectroscopic measurement of isotopic composition coupled with calorimetric measurement of total sample power is shown to give a totally nondestructive determination of sample plutonium mass with a precision of 0.6% for 1000-g samples of PuO/sub 2/ with 12% /sup 240/Pu content. The precision of isotopic measurements depends upon many factors, including sample size, sample geometry, and isotopic content. Typical ranges are found to be /sup 238/Pu, 1 to 10%; /sup 239/Pu, 0.1 to 0.5%; /sup 240/Pu, 2 to 5%; /sup 241/Pu, 0.3 to 0.7%; /sup 242/Pu (determined by isotopic correlation); and /sup 241/Am, 0.2 to 10%.

  7. Pileup recovery algorithms for digital gamma ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Mahmoud, I. I.; El Tokhy, M. S.; Konber, H. A.

    2012-09-01

    This paper presents algorithms for overcoming a common problem of gamma ray spectroscopy, namely the peak pileup recovery problem. Three different approaches are studied and evaluated within a spectroscopy system. The algorithms are evaluated by the means of parameters error and fitting error calculations. The first approach is a direct search based on Nelder-Mead technique without any derivatives in order to find the local minimum points. A Gaussian shape in conjunction with the peak height and its position of each pulse are used to construct the pulse. So, the main pulse parameters such as peak amplitude, position and width can be determined. The second algorithm is based on the nonlinear least square method. In this paper another technique is tried. This technique which is proposed as third algorithm is based on a maximum peak search method combined with the first derivative method to determine peak position of each pulse. Comparison among these approaches is conducted in terms of parameters errors. The pulse parameters have been calculated and compared with the actual one. The second approach shows the best accuracy, for determining peak height and position, but the width parameter scored the highest error.

  8. Bismuth-Loaded Polymer Scintillators for Gamma Ray Spectroscopy

    SciTech Connect

    Rupert, B L; Cherepy, N J; Sturm, B W; Sanner, R D; Dai, Z; Payne, S A

    2011-04-11

    We synthesize a series of polyvinylcarbazole monoliths containing varying loadings of triphenyl bismuth as a high-Z dopant and varying fluors, either organic or organometallic, in order to study their use as scintillators capable of gamma ray spectroscopy. A trend of increasing bismuth loading resulting in a better-resolved photopeak is observed. For PVK parts with no fluor or a standard organic fluor, diphenylanthracene, increasing bismuth loading results in decreasing light yield while with samples 1 or 3 % by weight of the spin-orbit coupling organometallic fluor FIrpic, which emits light from both singlet and triple excitons, show increasing light yield with increasing bismuth loading. Our best performing PVK/ BiPh{sub 3}/FIrpic scintillator with 40 wt % BiPh3 and 3 wt % FIrpic has an emission maximum of 500 nm, a light yield of {approx}30,000 photons/MeV, and energy resolution better than 7% FWHM at 662 keV. Replacing the Ir complex with an equal weight of diphenylanthracene produces a sample with a light yield of {approx}6,000 photons/MeV, with an emission maximum at 420 nm and energy resolution of 9% at 662 keV. Transmission electron microscopy studies show that the BiPh{sub 3} forms small clusters of approximately 5 nm diameter.

  9. Strontium Iodide Instrument Development for Gamma Spectroscopy and Radioisotope Identification

    SciTech Connect

    Beck, P; Cherepy, Nerine; Payne, Stephen A.; Swanberg, E.; Nelson, K.; Thelin, P; Fisher, S E; Hunter, Steve; Wihl, B; Shah, Kanai; Hawrami, Rastgo; Burger, Arnold; Boatner, Lynn A; Momayezi, M; Stevens, K; Randles, M H; Solodovnikov, D

    2014-01-01

    Development of the Europium-doped Strontium Iodide scintillator, SrI2(Eu), has progressed significantly in recent years. SrI2(Eu) has excellent material properties for gamma ray spectroscopy: high light yield (>80,000 ph/MeV), excellent light yield proportionality, and high effective atomic number (Z=49) for high photoelectric cross-section. High quality 1.5 and 2 diameter boules are now available due to rapid advances in SrI2(Eu) crystal growth. In these large SrI2(Eu) crystals, optical self-absorption by Eu2+ degrades the energy resolution as measured by analog electronics, but we mitigate this effect through on-the-fly correction of the scintillation pulses by digital readout electronics. Using this digital correction technique we have demonstrated energy resolution of 2.9% FWHM at 662 keV for a 4 in3 SrI2(Eu) crystal, over 2.6 inches long. Based on this digital readout technology, we have developed a detector prototype with greatly improved radioisotope identification capability compared to Sodium Iodide, NaI(Tl). The higher resolution of SrI2(Eu) yields a factor of 2 to 5 improvement in radioisotope identification (RIID) error rate compared to NaI(Tl).

  10. Decay Heat Measurements Using Total Absorption Gamma-ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Rice, S.; Valencia, E.; Algora, A.; Taín, J. L.; Regan, P. H.; Podolyák, Z.; Agramunt, J.; Gelletly, W.; Nichols, A. L.

    2012-09-01

    A knowledge of the decay heat emitted by thermal neutron-irradiated nuclear fuel is an important factor in ensuring safe reactor design and operation, spent fuel removal from the core, and subsequent storage prior to and after reprocessing, and waste disposal. Decay heat can be readily calculated from the nuclear decay properties of the fission products, actinides and their decay products as generated within the irradiated fuel. Much of the information comes from experiments performed with HPGe detectors, which often underestimate the beta feeding to states at high excitation energies. This inability to detect high-energy gamma emissions effectively results in the derivation of decay schemes that suffer from the pandemonium effect, although such a serious problem can be avoided through application of total absorption γ-ray spectroscopy (TAS). The beta decay of key radionuclei produced as a consequence of the neutron-induced fission of 235U and 239Pu are being re-assessed by means of this spectroscopic technique. A brief synopsis is given of the Valencia-Surrey (BaF2) TAS detector, and their method of operation, calibration and spectral analysis.

  11. Strontium iodide instrument development for gamma spectroscopy and radioisotope identification

    NASA Astrophysics Data System (ADS)

    Beck, P. R.; Cherepy, N. J.; Payne, S. A.; Swanberg, E. L.; Nelson, K. E.; Thelin, P. A.; Fisher, S. E.; Hunter, S.; Wihl, B. M.; Shah, K. S.; Hawrami, R.; Burger, A.; Boatner, L. A.; Momayezi, M.; Stevens, K. T.; Randles, M. H.; Solodovnikov, D.

    2014-09-01

    Development of the Europium-doped Strontium Iodide scintillator, SrI2(Eu2+), has progressed significantly in recent years. SrI2(Eu2+) has excellent material properties for gamma ray spectroscopy: high light yield (<80,000 ph/MeV), excellent light yield proportionality, and high effective atomic number (Z = 49) for high photoelectric cross-section. High quality 1.5" and 2" diameter boules are now available due to rapid advances in SrI2(Eu) crystal growth. In these large SrI2(Eu) crystals, optical self-absorption by Eu2+ degrades the energy resolution as measured by analog electronics, but we mitigate this effect through on-the-fly correction of the scintillation pulses by digital readout electronics. Using this digital correction technique we have demonstrated energy resolution of 2.9% FWHM at 662 keV for a 4 in3 SrI2(Eu) crystal, over 2.6 inches long. Based on this digital readout technology, we have developed a detector prototype with greatly improved radioisotope identification capability compared to Sodium Iodide, NaI(Tl). The higher resolution of SrI2(Eu) yields a factor of 2 to 5 improvement in radioisotope identification (RIID) error rate compared to NaI(Tl).

  12. Ultra-low background measurement capabilities at SNOLAB

    NASA Astrophysics Data System (ADS)

    Lawson, Ian

    2016-05-01

    Experiments currently searching for dark matter, studying properties of neutrinos or searching for neutrinoless double-beta decay require very low levels of radioactive backgrounds both in their own construction materials and in the surrounding environment. These low background levels are required so that the current generation of experiments can achieve the required sensitivities for their searches. SNOLAB has several facilities which are used to directly measure these radioactive backgrounds. This paper will describe SNOLAB’s ultra-low background germanium detectors, describe the data analysis techniques used and present results from these detectors. A description of SNOLAB’s alpha-beta and electrostatic counters will be presented and the underground low background counting laboratory currently under construction at SNOLAB will be presented.

  13. Neutron Spallation Measurements And Impacts On Low Background Experiments

    SciTech Connect

    Aguayo, Estanislao; Kouzes, Richard T.; Siciliano, Edward R.

    2014-09-01

    Ultra-low background experiments, such as neutrinoless double beta decay, carried out deep underground to escape cosmic ray backgrounds can nonetheless be limited in sensitivity by cosmogenically induced signals. This limit can either be produced directly during operation from cosmic muon events in the detector volume, or can be produced by radioactive decay of cosmogenically generated radionuclides created while the detector materials were above ground. An accurate knowledge of the production of the latter source of background is of paramount importance in order to be able to interpret the results of low-background experiments.

  14. Low-background temperature sensors fabricated on parylene substrates

    NASA Astrophysics Data System (ADS)

    Dhar, A.; Loach, J. C.; Barton, P. J.; Larsen, J. T.; Poon, A. W. P.

    2015-12-01

    Temperature sensors fabricated from ultra-low radioactivity materials have been developed for low-background experiments searching for neutrinoless double-beta decay and the interactions of WIMP dark matter. The sensors consist of electrical traces photolithographically-patterned onto substrates of vapor-deposited parylene. They are demonstrated to function as expected, to do so reliably and robustly, and to be highly radio-pure. This work is a proof-of-concept study of a technology that can be applied to broad class of electronic circuits used in low-background experiments.

  15. Design of a Low Background Liquid Scintillation Counter for a Shallow Underground Laboratory

    NASA Astrophysics Data System (ADS)

    Orrell, John; Aalseth, Craig; Bernacki, Bruce; Douglas, Matt; Erchinger, Jennifer; Fuller, Erin; Keillor, Martin; Morley, Shannon; Mullen, Crystal; Panisko, Mark; Shaff, Sarah; Warren, Glen; Wright, Michael

    2014-09-01

    Pacific Northwest National Laboratory operates a 35-meter water-equivalent overburden, shallow underground laboratory for measuring low-concentration radioactive isotopes in environmental samples collected. A low-background liquid scintillation counter is under development. Liquid scintillation counting is useful for beta-emitting isotopes without (or low) gamma ray yields. The high-efficiency beta detection in a liquid scintillation cocktail coupled with the low-background environment of a shield located in a clean underground laboratory provides for increased-sensitivity measurements to a range of isotopes. Benchmarked simulations have evaluated the shield design requirements to assess the background rate achievable. Assay of shield construction materials provides the basis for the shield design development. The low background design is informed by efforts in experimental design of neutrinoless double beta decay experiments, direct detection dark matter experiments, and low energy neutrino detection experiments. In this vein a background budget for the instrument is presented with attention to low background methods directed toward applications of nuclear measurements.

  16. Detector arrays for low-background space infrared astronomy

    NASA Technical Reports Server (NTRS)

    Mccreight, C. R.; Mckelvey, M. E.; Goebel, J. H.; Anderson, G. M.; Lee, J. H.

    1986-01-01

    The status of development and characterization tests of integrated infrared detector array technology for astronomy applications is described. The devices under development include intrinsic, extrinsic silicon, and extrinsic germanium detectors, with hybrid silicon multiplexers. Laboratary test results and successful astronomy imagery have established the usefulness of integrated arrays in low-background astronomy applications.

  17. Detector arrays for low-background space infrared astronomy

    NASA Technical Reports Server (NTRS)

    Mccreight, C. R.; Mckelvey, M. E.; Goebel, J. H.; Anderson, G. M.; Lee, J. H.

    1986-01-01

    The status of development and characterization tests of integrated infrared detector array technology for astronomy applications is described. The devices under development include intrinsic, extrinsic silicon, and extrinsic germanium detectors, with hybrid silicon multiplexers. Laboratory test results and successful astronomy imagery have established the usefulness of integrated arrays in low-background astronomy applications.

  18. Gamma-ray/neutron spectroscopy from the Mars observer

    NASA Technical Reports Server (NTRS)

    Englert, P.; Reedy, R. C.; Drake, D. M.; Feldman, W. C.; Squyres, S. W.; Evans, L. G.; Boynton, W. V.

    1987-01-01

    The Gamma-Ray Spectrometer (GRS) experiment on Mars Observer will measure gamma rays and neutrons that escape from Mars. The intensities of gamma-ray lines and of the thermal and epithermal neutrons can be used to study many problems related to Martian volcanism and volatiles. The results of theoretical calculations for the production and transport of gamma rays and neutrons indicate that the GRS should be able to determine the abundances of many elements and the amounts and stratigraphy of H2O and CO2 on and in the top meter of the Martian surface. Design considerations of the GRS are discussed.

  19. Abundances from solar-flare gamma-ray line spectroscopy

    NASA Technical Reports Server (NTRS)

    Murphy, R. J.; Ramaty, R.; Forrest, D. J.; Kozlovsky, B.

    1985-01-01

    Elemental abundances of the ambient gas at the site of gamma ray line production inthe solar atmosphere are deduced using gamma ray line observations from a solar flare. The resultant abundances are different from local galactic abundances which are thought to be similar to photospheric abundances.

  20. The goals of gamma-ray spectroscopy in high energy astrophysics

    NASA Technical Reports Server (NTRS)

    Lingenfelter, Richard E.; Higdon, James C.; Leventhal, Marvin; Ramaty, Reuven; Woosley, Stanford E.

    1990-01-01

    The use of high resolution gamma-ray spectroscopy in astrophysics is discussed with specific attention given to the application of the Nuclear Astrophysics Explorer (NAE). The gamma-ray lines from nuclear transitions in radionucleic decay and positron annihilation permits the study of current sites, rates and models of nucleosynthesis, and galactic structure. Diffuse galactic emission is discussed, and the high-resolution observations of gamma-ray lines from discrete sites are also described. Interstellar mixing and elemental abundances can also be inferred from high-resolution gamma-ray spectroscopy of nucleosynthetic products. Compact objects can also be examined by means of gamma-ray emissions, allowing better understanding of neutron stars and the accreting black hole near the galactic center. Solar physics can also be investigated by examining such features as solar-flare particle acceleration and atmospheric abundances.

  1. The goals of gamma-ray spectroscopy in high energy astrophysics

    NASA Astrophysics Data System (ADS)

    Lingenfelter, Richard E.; Higdon, James C.; Leventhal, Marvin; Ramaty, Reuven; Woosley, Stanford E.

    1990-08-01

    The use of high resolution gamma-ray spectroscopy in astrophysics is discussed with specific attention given to the application of the Nuclear Astrophysics Explorer (NAE). The gamma-ray lines from nuclear transitions in radionucleic decay and positron annihilation permits the study of current sites, rates and models of nucleosynthesis, and galactic structure. Diffuse galactic emission is discussed, and the high-resolution observations of gamma-ray lines from discrete sites are also described. Interstellar mixing and elemental abundances can also be inferred from high-resolution gamma-ray spectroscopy of nucleosynthetic products. Compact objects can also be examined by means of gamma-ray emissions, allowing better understanding of neutron stars and the accreting black hole near the galactic center. Solar physics can also be investigated by examining such features as solar-flare particle acceleration and atmospheric abundances.

  2. Planetary gamma-ray spectroscopy. [for element distribution over planetary surfaces

    NASA Technical Reports Server (NTRS)

    Reedy, R. C.

    1978-01-01

    The measured intensities of certain gamma rays of specific energies escaping from a planetary surface can be used to determine the abundances of a number of elements. The fluxes of the more intense gamma ray lines emitted from 32 elements have been calculated using current nuclear data and existing models for the source processes. The fluxes emitted from a surface of average lunar composition are reported for 292 gamma ray lines. Detection sensitivities for various elements are examined and applications of gamma ray spectroscopy for future orbiters to Mars and other solar system objects are discussed.

  3. Quantum Well Infrared Photodetectors for Low Background Applications

    NASA Technical Reports Server (NTRS)

    Gunapala, S. D.; Bandara, S. V.; Singh, A.; Liu, J. K.; Luong, E. M.; Mumolo, J. M.; McKelvey, M. J.

    1998-01-01

    High performance long-wavelength GaAs/Al(x)Ga(1-x)As quantum well infrared photodetectors for low background applications have been demonstrated. This is the first theoretical analysis of quantum well infrared photodetectors for low background applications and the detectivity D* of 6 x 10(exp 13) cm.square root of Hz/W has been achieved at T = 40 K with 2 x 10(exp 9) photons/cm2/sec background. In addition, this paper describes the demonstration of mid-wavelength/long-wavelength dualband quantum well infrared photodetectors and long-wavelength/very long-wavelength dualband quantum well infrared photodetectors in 4-26 micrometers wavelength region.

  4. Low background HPGe spectrometer in investigations of 2β decay

    SciTech Connect

    Rukhadze, Ekaterina [Institute of Experimental and Applied Physics, CTU in Prague, Horska 3a Collaboration: OBELIX Collaboration; TGV Collaboration; SuperNEMO Collaboration; and others

    2013-08-08

    The low background high sensitive HPGe spectrometer called OBELIX is briefly described. The calibration measurements using {sup 152}Eu, {sup 133}Ba and La{sub 2}O{sub 3} sources in different geometries, the obtained efficiency curves for OBELIX HPGe detector, the results of measurements of radioactivity of the NEMO-3 sources ({sup 100}Mo, {sup 150}Nd) as well as future plans for OBELIX detector (e.g. 0νEC/EC decay of {sup 106}Cd) are presented.

  5. Design Considerations for Large Mass Ultra-Low Background Experiments

    SciTech Connect

    Aguayo Navarrete, Estanislao; Reid, Douglas J.; Fast, James E.; Orrell, John L.

    2011-07-01

    Summary The objective of this document is to present the designers of the next generation of large-mass, ultra-low background experiments with lessons learned and design strategies from previous experimental work. Design issues divided by topic into mechanical, thermal and electrical requirements are addressed. Large mass low-background experiments have been recognized by the scientific community as appropriate tools to aid in the refinement of the standard model. The design of these experiments is very costly and a rigorous engineering review is required for their success. The extreme conditions that the components of the experiment must withstand (heavy shielding, vacuum/pressure and temperature gradients), in combination with unprecedented noise levels, necessitate engineering guidance to support quality construction and safe operating conditions. Physical properties and analytical results of typical construction materials are presented. Design considerations for achieving ultra-low-noise data acquisition systems are addressed. Five large-mass, low-background conceptual designs for the one-tonne scale germanium experiment are proposed and analyzed. The result is a series of recommendations for future experiments engineering and for the Majorana simulation task group to evaluate the different design approaches.

  6. GeMSE: A new low-background facility for meteorite and material screening

    NASA Astrophysics Data System (ADS)

    Sivers, M. V.; Hofmann, B. A.; Rosén, Å. V.; Schumann, M.

    2015-08-01

    We are currently setting up a facility for low-background gamma-ray spectrometry based on a HPGe detector. It is dedicated to material screening for the XENON and DARWIN dark matter projects as well as to the characterization of meteorites. The detector will be installed in a medium depth (˜620 m.w.e.) underground laboratory in Switzerland with several layers of shielding and an active muon-veto. The GeMSE facility will be operational by fall 2015 with an expected background rate of ˜250 counts/day (100-2700 keV).

  7. Sub-Kelvin Thermal Conductivity and Radioactivity of Some Useful Materials in Low Background Cryogenic Experiments

    NASA Astrophysics Data System (ADS)

    Kellaris, N.; Daal, M.; Epland, M.; Pepin, M.; Kamaev, O.; Cushman, P.; Kramer, E.; Sadoulet, B.; Mirabolfathi, N.; Golwala, S.; Runyan, M.

    2014-08-01

    We present measurements of the thermal conductivity between 0.05 and 1 K, and radioactive contamination levels, for some thermally isolating materials. TIMET Ti 15-3-3-3, Mersen grade 2020 graphite, Vespel SP-1, Vespel SP-22, Vespel SCP-5000, Vespel SCP-5050, Graphlite CFRP, and a Kapton/epoxy composite are all investigated. Thermal conductivities were measured using a single-heater longitudinal heat flow method. Material radioactivity was determined for the materials at a low background counting facility using a high-purity gamma detector and GEANT4 Monte Carlo simulations.

  8. Gamma ray production cross section from energetic neutron inelastic scattering for methodical improvements in planetary gamma-ray spectroscopy

    SciTech Connect

    Castaneda, C.M.; Gearhart, R.; Sanii, B.; Englert, P.A.J.; Drake, D.M.; Reedy, R.C.

    1991-12-31

    Planetary Gamma ray spectroscopy can be used to chemically analyze the top soil from planets in future planetary missions. The production from inelastic neutron interaction plays an effective role in the determination on the C and H at the surface. The gamma ray production cross section from the strongest lines excited in the neutron bombardment of Fe have been measured by the use of a time analyzed quasi-mono-energetic neutron beam and a high purity germanium detector. The results from En=6.5, 32, 43, and 65 MeV are presented.

  9. The Northern Marshall Islands radiological survey: A quality control program for radiochemical and gamma spectroscopy analysis

    SciTech Connect

    Kehl, S.R.; Mount, M.E.; Robison, W.L.

    1995-09-01

    From 1979 to 1989, approximately 25,000 Post Northern Marshall Islands Radiological Survey (PNMIRS) samples were collected, and over 71,400 radiochemical and gamma spectroscopy analyses were performed to establish the concentration of {sup 90}Sr, {sup 137}Cs, {sup 241}Am, and plutonium isotopes in soil, vegetation, fish, and animals in the Northern Marshall Islands. While the Low Level Gamma Counting Facility (B379) in the Health and Ecological Assessment (HEA) division accounted for over 80% of all gamma spectroscopy analyses, approximately 4889 radiochemical and 5437 gamma spectroscopy analyses were performed on 4784 samples of soil, vegetation, terrestrial animal, and marine organisms by outside laboratories. Four laboratories were used by Lawrence Livermore National Laboratory (LLNL) to perform the radiochemical analyses: Thermo Analytical Norcal, Richmond, California (TMA); Nuclear Energy Services, North Carolina State University (NCSU); Laboratory of Radiation Ecology, University of Washington (LRE); and Health and Ecological Assessment (HEA) division, LLNL, Livermore, California. Additionally, LRE and NCSU were used to perform gamma spectroscopy analyses. The analytical precision and accuracy were monitored by including blind duplicates and natural matrix standards in each group of samples analyzed. On the basis of reported analytical values for duplicates and standards, 88% of the gamma and 87% of the radiochemical analyses in this survey were accepted. By laboratory, 93% of the radiochemical analyses by TMA; 88% of the gamma-ray spectrometry and 100% of the radiochemistry analyses by NCSU; 89% of the gamma spectroscopy and 87% of the radiochemistry analyses by LRE; and 90% of the radiochemistry analyses performed by HEA`s radiochemistry department were accepted.

  10. Development of a low background liquid scintillation counter for a shallow underground laboratory

    SciTech Connect

    Erchinger, Jennifer L.; Aalseth, Craig E.; Bernacki, Bruce E.; Douglas, Matthew; Fuller, Erin S.; Keillor, Martin E.; Morley, Shannon M.; Mullen, Crystal A.; Orrell, John L.; Panisko, Mark E.; Warren, Glen A.; Williams, Russell O.; Wright, Michael E.

    2015-08-20

    Pacific Northwest National Laboratory has recently opened a shallow underground laboratory intended for measurement of lowconcentration levels of radioactive isotopes in samples collected from the environment. The development of a low-background liquid scintillation counter is currently underway to further augment the measurement capabilities within this underground laboratory. Liquid scintillation counting is especially useful for measuring charged particle (e.g., B, a) emitting isotopes with no (orvery weak) gamma-ray yields. The combination of high-efficiency detection of charged particle emission in a liquid scintillation cocktail coupled with the low-background environment of an appropriately-designed shield located in a clean underground laboratory provides the opportunity for increased-sensitivity measurements of a range of isotopes. To take advantage of the 35-meter water-equivalent overburden of the underground laboratory, a series of simulations have evaluated the instrumental shield design requirements to assess the possible background rate achievable. This report presents the design and background evaluation for a shallow underground, low background liquid scintillation counter design for sample measurements.

  11. Development of a low background liquid scintillation counter for a shallow underground laboratory.

    PubMed

    Erchinger, J L; Aalseth, C E; Bernacki, B E; Douglas, M; Fuller, E S; Keillor, M E; Morley, S M; Mullen, C A; Orrell, J L; Panisko, M E; Warren, G A; Williams, R O; Wright, M E

    2015-11-01

    Pacific Northwest National Laboratory has recently opened a shallow underground laboratory intended for measurement of low-concentration levels of radioactive isotopes in samples collected from the environment. The development of a low-background liquid scintillation counter is currently underway to further augment the measurement capabilities within this underground laboratory. Liquid scintillation counting is especially useful for measuring charged particle (e.g., β and α) emitting isotopes with no (or very weak) gamma-ray yields. The combination of high-efficiency detection of charged particle emission in a liquid scintillation cocktail coupled with the low-background environment of an appropriately designed shield located in a clean underground laboratory provides the opportunity for increased-sensitivity measurements of a range of isotopes. To take advantage of the 35m-water-equivalent overburden of the underground laboratory, a series of simulations have evaluated the scintillation counter's shield design requirements to assess the possible background rate achievable. This report presents the design and background evaluation for a shallow underground, low background liquid scintillation counter design for sample measurements. PMID:26334781

  12. CASCADES: An Ultra-Low-Background Germanium Crystal Array at Pacific Northwest National Laboratory

    NASA Astrophysics Data System (ADS)

    Keillor, M. E.; Aalseth, C. E.; Day, A. R.; Erikson, L. E.; Fast, J. E.; Glasgow, B. D.; Hoppe, E. W.; Hossbach, T. W.; Hyronimus, B. J.; Miley, H. S.; Myers, A. W.; Seifert, A.; Stavenger, T. J.

    2011-12-01

    State-of-the-art treaty verification techniques, environmental surveillance, and physics experiments require increased sensitivity for detecting and quantifying radionuclides of interest. This can be accomplished with new detector designs that establish high detection efficiency and reduced instrument backgrounds. Current research is producing an intrinsic germanium (HPGe) array designed for high detection efficiency, ultra-low-background performance, and sensitive γ—γ coincidence detection. The system design is optimized to accommodate filter paper samples, e.g. samples collected by the Radionuclide Aerosol Sampler/Analyzer. The system will provide high sensitivity for weak collections on atmospheric filter samples (e.g.<105 fissions) as well as offering the potential to gather additional information from higher activity filters using gamma cascade coincidence detection. The first of two HPGe crystal arrays in ultra-low-background vacuum cryostats has been assembled, with the second in progress. Traditional methods for constructing ultra-low-background detectors were followed, including use of materials known to be low in radioactive contaminants, use of ultra-pure reagents, and clean room assembly. The cryostat is constructed mainly from copper electroformed into near-final geometry at Pacific Northwest National Laboratory. Details of the detector assembly and initial background and spectroscopic measurement results are presented; also a description of the custom analysis package used by this project is given.

  13. Neutron counting and gamma spectroscopy with PVT detectors.

    SciTech Connect

    Mitchell, Dean James; Brusseau, Charles A.

    2011-06-01

    Radiation portals normally incorporate a dedicated neutron counter and a gamma-ray detector with at least some spectroscopic capability. This paper describes the design and presents characterization data for a detection system called PVT-NG, which uses large polyvinyl toluene (PVT) detectors to monitor both types of radiation. The detector material is surrounded by polyvinyl chloride (PVC), which emits high-energy gamma rays following neutron capture reactions. Assessments based on high-energy gamma rays are well suited for the detection of neutron sources, particularly in border security applications, because few isotopes in the normal stream of commerce have significant gamma ray yields above 3 MeV. Therefore, an increased count rate for high-energy gamma rays is a strong indicator for the presence of a neutron source. The sensitivity of the PVT-NG sensor to bare {sup 252}Cf is 1.9 counts per second per nanogram (cps/ng) and the sensitivity for {sup 252}Cf surrounded by 2.5 cm of polyethylene is 2.3 cps/ng. The PVT-NG sensor is a proof-of-principal sensor that was not fully optimized. The neutron detector sensitivity could be improved, for instance, by using additional moderator. The PVT-NG detectors and associated electronics are designed to provide improved resolution, gain stability, and performance at high-count rates relative to PVT detectors in typical radiation portals. As well as addressing the needs for neutron detection, these characteristics are also desirable for analysis of the gamma-ray spectra. Accurate isotope identification results were obtained despite the common impression that the absence of photopeaks makes data collected by PVT detectors unsuitable for spectroscopic analysis. The PVT detectors in the PVT-NG unit are used for both gamma-ray and neutron detection, so the sensitive volume exceeds the volume of the detection elements in portals that use dedicated components to detect each type of radiation.

  14. Material Analysis/Characterization for Ultra-Low Background Experiments

    NASA Astrophysics Data System (ADS)

    Jasinski, Ben

    For the discovery of rare event physics processes related to new physics beyond the Standard Model, the next generation of physics experiments requires to be built underground. For instance, the Large Underground Xenon experiment and MAJORANA DEMONSTRATOR, both located underground at the Sanford Underground Research Facility (SURF), require an ultra-low background rate for their respective discovery of Dark Matter and the Majorana particle. The next generation of detectors designated for these ultra-low background experiments require a complete understanding of the materials used in the experiment to achieve the detection sensitivity below the current limits. Experimental limits can be seen in ton scale detector designs where ultrapure materials are needed for detector performance, suppression of background radiation, and electronic noise. This thesis studies the three main aspects of ultra-low background experiments. First, an investigation of the mechanical design constraints for SURF underground physics experiments is performed. Second, a study into each detector's characterization and performance is described for the SURF experiments. Lastly, an optimization of data analysis algorithm for rare event physics is discussed. We describe the techniques used for the above three investigations in detail. First, the test of the mechanical design constraints is investigated using an adaptive sample holder capable of testing sample materials of gas, liquid or solid state. Second, the characterization of materials is studied with a design of a Capacitance-Voltage Measurement system. Lastly, the optimization of data analysis algorithm for small signals is performed by a detailed data analysis to verify isotopic enrichment obtained from a novel isotope separation method of molecules of CO2.

  15. Low background techniques for the Borexino nylon vessels

    SciTech Connect

    Pocar, Andrea

    2005-09-08

    Borexino is an organic liquid scintillator underground detector for low energy solar neutrinos. The experiment has to satisfy extremely stringent low background requirements. The thin nylon spherical scintillator containment vessel has to meet cleanliness and low radioactivity levels second only, within the detector, to the scintillator itself. Overall, the background from the vessel in the fiducial volume of the detector must be kept at the level of one event per day or better. The requirements, design choices, results from laboratory tests, and fabrication techniques that have been adopted to meet this goal are presented. Details of the precautions taken during the installation of the vessels inside the Borexino detector are also discussed.

  16. LWIR detector requirements for low-background space applications

    NASA Technical Reports Server (NTRS)

    Deluccia, Frank J.

    1990-01-01

    Detection of cold bodies (200 to 300 K) against space backgrounds has many important applications, both military and non-military. The detector performance and design characteristics required to support low-background applications are discussed, with particular emphasis on those characteristics required for space surveillance. The status of existing detector technologies under active development for these applications is also discussed. In order to play a role in future systems, new, potentially competing detector technologies such as multiple quantum well detectors must not only meet system-derived requirements, but also offer distinct performance or other advantages over these incumbent technologies.

  17. Experimental approaches for the development of gamma spectroscopy well logging system

    SciTech Connect

    Shin, Jehyun; Hwang, Seho; Kim, Jongman; Won, Byeongho

    2015-03-10

    This article discusses experimental approaches for the development of gamma spectroscopy well logging system. Considering the size of borehole sonde, we customize 2 x 2 inches inorganic scintillators and the system including high voltage, preamplifier, amplifier and multichannel analyzer (MCA). The calibration chart is made by test using standard radioactive sources so that the measured count rates are expressed by energy spectrum. Optimum high-voltage supplies and the measurement parameters of each detector are set up by experimental investigation. Also, the responses of scintillation detectors have been examined by analysis according to the distance between source and detector. Because gamma spectroscopy well logging needs broad spectrum, high sensitivity and resolution, the energy resolution and sensitivity as a function of gamma ray energy are investigated by analyzing the gamma ray activities of the radioactive sources.

  18. Feasibility study of plutonium isotopic analysis of resin beads by nondestructive gamma-ray spectroscopy

    SciTech Connect

    Li, T.K.

    1985-01-01

    We have initiated a feasibility study on the use of nondestructive low-energy gamma-ray spectroscopy for plutonium isotopic analysis on resin beads. Seven resin bead samples were measured, with each sample containing an average of 9 ..mu..g of plutonium; the isotopic compositions of the samples varied over a wide range. The gamma-ray spectroscopy results, obtained from 4-h counting-time measurements, were compared with mass spectrometry results. The average ratios of gamma-ray spectroscopy to mass spectrometry were 1.014 +- 0.025 for /sup 238/Pu//sup 239/Pu, 0.996 +- 0.018 for /sup 240/Pu//sup 239/Pu, and 0.980 +- 0.038 for /sup 241/Pu//sup 239/Pu. The rapid, automated, and accurate nondestructive isotopic analysis of resin beads may be very useful to process technicians and International Atomic Energy Agency inspectors. 3 refs., 1 fig., 3 tabs.

  19. Effects of material mixing on planetary gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Squyres, Steven W.; Evans, Larry G.

    1992-01-01

    The effect of mixing of rocks and soil on the gamma-ray signal emitted by Martian surface was investigated with special consideration given to the effect of the geometry of mixing. It is shown that, under certain circumstances, this scale can have a significant effect on the gamma-ray spectrum observed. The techniques that can be used to address this problem are discussed, showing that, using these techniques, rock compositions can be inferred from the signal produced by a rock-soil mixtures of unknown rock concentration and mixing geometry.

  20. Solar neon abundances from gamma-ray spectroscopy and He-3-rich particle events

    NASA Technical Reports Server (NTRS)

    Reames, D. V.; Ramaty, R.; Von Rosenvinge, T. T.

    1988-01-01

    Ambient solar atmospheric abundances derived from gamma-ray spectroscopy are compared with observations of solar energetic particles. Agreement is found between the gamma-ray-derived Ne/O ratio and the corresponding mean ratio for He-3-rich flares. Both of these values are significantly higher than inferred coronal Ne/O ratios. It is suggested that the mean Ne/O ratio in He-3-rich flares reflects the composition of the flare plasma rather than the acceleration process.

  1. A simple technique for gamma ray and cosmic ray spectroscopy using plastic scintillator

    NASA Astrophysics Data System (ADS)

    Nandan, Akhilesh P.; Rudra, Sharmili; Neog, Himangshu; Biswas, S.; Mahapatra, S.; Mohanty, B.; Samal, P. K.

    2016-07-01

    A new and simple technique has been developed using plastic scintillator detectors for gamma ray and cosmic ray spectroscopy without single channel analyzer (SCA) or multichannel analyzer (MCA). In these experiments only a leading edge discriminator (LED) and NIM scalers have been used. Energy calibration of gamma spectra in plastic scintillators has been done using Co60 and Cs137 sources. The details of the experimental technique, analysis procedure and experimental results have been presented in this paper.

  2. The ultra-pure Ti for the low background experiments

    SciTech Connect

    Chepurnov, Alexander; Nisi, Stefano; Vacri, Maria Laura di; Suvorov, Yury

    2013-08-08

    The constant increase in mass of the cryostats, containment tanks, passive shielding and other mechanical elements of the modern low background detectors put more stringent requirements on their radiopurity levels. In general they have to be ∼1 mBq/kg of {sup 238}U/{sup 232}Th or lower, which means that mass concentration should be < 0.1 ppb for {sup 238}U and < 0.25 ppb for {sup 232}Th. Traditionally, the field relies on specially selected low background stainless steel, electrochemical oxygen-free copper, or a combination of the two. However, the most promising material in terms of physical and mechanical properties is Titanium. Our study of various Ti samples show that the levels of contaminations of commercially available industrial titanium can varies from 0.2 to 100 mBq/kg for U/Th. Therefore, the only possible way to obtain the material with a low and controlled level of contamination is to develop (or improve the existing) the production technology and to build the dedicated manufactory line.

  3. In situ gamma-ray spectrometry in the environment using dose rate spectroscopy

    NASA Astrophysics Data System (ADS)

    Ji, Young-Yong; Kim, Chang-Jong; Chung, Kun Ho; Choi, Hee-Yeoul; Lee, Wanno; Kang, Mun Ja; Park, Sang Tae

    2016-02-01

    In order to expand the application of dose rate spectroscopy to the environment, in situ gamma-ray spectrometry was first conducted at a height of 1 m above the ground to calculate the ambient dose rate and individual dose rate at that height, as well as the radioactivity in the soil layer for the detected gamma nuclides from the dose rate spectroscopy. The reliable results could be obtained by introducing the angular correction factor to correct the G-factor with respect to incident photons distributed in a certain range of angles. The intercomparison results of radioactivity using ISOCS software, an analysis of a sample taken from the soil around a detector, and dose rate spectroscopy had a difference of <20% for 214Pb, 214Bi, 228Ac, 212Bi, 208Tl, and 40K, except for 212Pb with low-energy photons, that is, <300 keV. In addition, the drawback of using dose rate spectroscopy, that is, all gamma rays from a nuclide should be identified to accurately assess the individual dose rate, was overcome by adopting the concept of contribution ratio of the key gamma ray to the individual dose rate of a nuclide, so that it could be accurately calculated by identifying only a key gamma ray from a nuclide.

  4. Proton range verification through prompt gamma-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Verburg, Joost M.; Seco, Joao

    2014-12-01

    We present an experimental study of a novel method to verify the range of proton therapy beams. Differential cross sections were measured for 15 prompt gamma-ray lines from proton-nuclear interactions with 12C and 16O at proton energies up to 150 MeV. These cross sections were used to model discrete prompt gamma-ray emissions along proton pencil-beams. By fitting detected prompt gamma-ray counts to these models, we simultaneously determined the beam range and the oxygen and carbon concentration of the irradiated matter. The performance of the method was assessed in two phantoms with different elemental concentrations, using a small scale prototype detector. Based on five pencil-beams with different ranges delivering 5 × 108 protons and without prior knowledge of the elemental composition at the measurement point, the absolute range was determined with a standard deviation of 1.0-1.4 mm. Relative range shifts at the same dose level were detected with a standard deviation of 0.3-0.5 mm. The determined oxygen and carbon concentrations also agreed well with the actual values. These results show that quantitative prompt gamma-ray measurements enable knowledge of nuclear reaction cross sections to be used for precise proton range verification in the presence of tissue with an unknown composition.

  5. Gamma-ray spectroscopy of neutron-rich products of heavy-ion collisions

    SciTech Connect

    Carpenter, M.P.; Janssens, R.V.F.; Ahmad, I.

    1995-08-01

    Thick-target {gamma}{gamma} coincidence techniques are being used to explore the spectroscopy of otherwise hard-to-reach neutron-rich products of deep-inelastic heavy ion reactions. Extensive {gamma}{gamma} coincidence measurements were performed at ATLAS using pulsed beams of {sup 80}Se, {sup 136}Xe, and {sup 238}U on lead-backed {sup 122,124}Sn targets with energies 10-15% above the Coulomb barrier. Gamma-ray coincidence intensities were used to map out yield distributions with A and Z for even-even product nuclei around the target and around the projectile. The main features of the yield patterns are understandable in terms of N/Z equilibration. We had the most success in studying the decays of yrast isomers. Thus far, more than thirty new {mu}s isomers in the Z = 50 region were found and characterized. Making isotopic assignments for previously unknown {gamma}-ray cascades proves to be one of the biggest problems. Our assignments were based (a) on rare overlaps with radioactivity data, (b) on the relative yields with different beams, and (c) on observed cross-coincidences between {gamma} rays from light and heavy reaction partners. However, the primary products of deep inelastic collisions often are sufficiently excited for subsequent neutron evaporation, so {gamma}{gamma} cross-coincidence results require careful interpretation.

  6. Radiation detection system for portable gamma-ray spectroscopy

    DOEpatents

    Rowland, Mark S.; Howard, Douglas E.; Wong, James L.; Jessup, James L.; Bianchini, Greg M.; Miller, Wayne O.

    2006-06-20

    A portable gamma ray detection apparatus having a gamma ray detector encapsulated by a compact isolation structure having at least two volumetrically-nested enclosures where at least one is a thermal shield. The enclosures are suspension-mounted to each other to successively encapsulate the detector without structural penetrations through the thermal shields. A low power cooler is also provided capable of cooling the detector to cryogenic temperatures without consuming cryogens, due to the heat load reduction by the isolation structure and the reduction in the power requirements of the cooler. The apparatus also includes a lightweight portable power source for supplying power to the apparatus, including to the cooler and the processing means, and reducing the weight of the apparatus to enable handheld operation or toting on a user's person.

  7. Instrument Development and Gamma Spectroscopy with Strontium Iodide

    SciTech Connect

    Cherepy, Nerine; Payne, Stephen A.; Sturm, Benjamin; Drury, Owen; O’Neal, S P; Thelin, P; Shah, Kanai; Hawrami, Rastgo; Momayezi, M; Hurst, B.; Wiggen, B.; Bhattacharya, P.; Burger, Arnold; Boatner, Lynn A; Ramey, Joanne Oxendine

    2012-01-01

    Development of the Europium-doped Strontium Iodide scintillator, SrI2(Eu), involves advances in crystal growth, optics and readout methodology for prototype detectors. We have demonstrated energy resolution of 3% at 662 keV for a 26 cm3 SrI2(Eu) crystal, which is comparable to the performance obtained with Cerium-doped Lanthanum Bromide of equivalent size. Compared to standard analog readout, use of a digital readout method allows improved energy resolution to be obtained with large-volume SrI2(Eu) crystals. Comparative gamma spectra acquired with LaBr3(Ce) and NaI(Tl) quantitatively depict the value of the high resolution and low intrinsic radioactivity of SrI2(Eu) in discriminating closely spaced gamma lines for radioisotope identification applications.

  8. Gamma ray spectroscopy in astrophysics: Future role of scintillation detectors

    NASA Technical Reports Server (NTRS)

    Kurfess, J. D.

    1978-01-01

    The future role of conventional scintillation detector telescopes for line gamma-ray astronomy is discussed. Although the energy resolution of the germanium detectors now being used by several groups is clearly desirable, the larger effective areas and higher efficiencies available with scintillation detectors is advantageous for many observations. This is particularly true for those observations of astrophysical phenomena where significant line broadening is expected.

  9. Gamma ray spectroscopy in astrophysics: Solar gamma ray astronomy on solar maximum mission. [experimental design

    NASA Technical Reports Server (NTRS)

    Forrest, D. J.

    1978-01-01

    The SMM gamma ray experiment and the important scientific capabilities of the instrument are discussed. The flare size detectable as a function of spectrum integration time was studied. A preliminary estimate indicates that a solar gamma ray line at 4.4 MeV one-fifth the intensity of that believed to have been emitted on 4 August 1972 can be detected in approximately 1000 sec with a confidence level of 99%.

  10. Characterization and modeling of a low background HPGe detector

    NASA Astrophysics Data System (ADS)

    Dokania, N.; Singh, V.; Mathimalar, S.; Nanal, V.; Pal, S.; Pillay, R. G.

    2014-05-01

    A high efficiency, low background counting setup has been made at TIFR consisting of a special HPGe detector (~ 70 %) surrounded by a low activity copper+lead shield. Detailed measurements are performed with point and extended geometry sources to obtain a complete response of the detector. An effective model of the detector has been made with GEANT4 based Monte Carlo simulations which agrees with experimental data within 5%. This setup will be used for qualification and selection of radio-pure materials to be used in a cryogenic bolometer for the study of Neutrinoless Double Beta Decay in 124Sn as well as for other rare event studies. Using this setup, radio-impurities in the rock sample from India-based Neutrino Observatory (INO) site have been estimated.

  11. The BiPo low-background detector project

    NASA Astrophysics Data System (ADS)

    Vasilyev, R. V.

    2009-05-01

    A low-background detector designed to search for weak radioactive pollution by 208Tl and 214Bi in thin samples of a large area is described. The samples are 12-m2 source foils made of 82Se or 150Nd enriched isotopes. Such samples are planned for use in investigating neutrinoless double β decay in the SuperNEMO experiment. The principle of the detector operation is based on registering the delayed β-α coincidence from the uranium and thorium radioactive chains. The sensitivity of the detector is planned to be at the level of 208Tl < 2 μBq/kg and 214Bi < 10 μBq/kg. Alternate versions of the detector are described. The first results obtained by the prototype detector, operated in the Frejus Underground Laboratory in France, are presented.

  12. Radiation shielding for underground low-background experiments

    SciTech Connect

    Stewart, D. Y.; Harrison, P. F.; Morgan, B.; Ramachers, Y.

    2006-11-17

    The design task of creating an efficient radiation shield for the new COBRA double-beta decay experiment led to a comprehensive study of commercially available shielding materials. The aim was to find the most efficient combination of materials under the constraints of an extreme low-background experiment operating in a typical underground laboratory. All existing shield configurations for this type of experiment have been found to perform sub-optimally in comparison to the class of multilayered configurations proposed in this study. The method used here to create a specific shield configuration should yield a close to optimal result when applied to any experiment utilising a radiation shield. In particular, the survey of single material response to a given radiation source turns out to give a guideline for the construction of efficient multilayer shields. Note that these proceedings are a short version of a recently submitted, more detailed discussion.

  13. High resolution {gamma}-ray spectroscopy: The first 85 years

    SciTech Connect

    Deslattes, R.D.

    2000-02-01

    This opening review attempts to follow the main trends in crystal diffraction spectrometry of nuclear {gamma} rays from its 1914 beginning in Rutherford's laboratory to the ultra-high resolution instrumentation realized in the current generation of spectrometers at the Institute Laue Langeven (ILL). The authors perspective is that of an instrumentalist hoping to convey a sense of intellectual debt to a number of predecessors, each of whom realized a certain elegance in making the tools that have enabled much good science, including that to which the remainder of this workshop is dedicated. This overview follows some of the main ideas along a trajectory toward higher resolution at higher energies, thereby enabling not only the disentangling of dense spectra, but also allowing detailed study of aspects of spectral profiles sensitive to excited state lifetimes and interatomic potentials. The parallel evolution toward increasing efficiency while preserving needed resolution is also an interesting story of artful compromise that should not be neglected. Finally, it is the robustness of the measurement chain connecting {gamma}-ray wavelengths with optical wave-lengths associated with the Rydberg constant that only recently has allowed {gamma}-ray data to contribute to determine of particle masses and fundamental constants, as will be described in more detail in other papers from this workshop.

  14. {gamma}-ray spectroscopy of {sup 197}At

    SciTech Connect

    Andgren, K.; Cederwall, B.; Baeck, T.; Hadinia, B.; Johnson, A.; Khaplanov, A.; Sandzelius, M.; Wyss, R.; Jakobsson, U.; Uusitalo, J.; Greenlees, P. T.; Jones, P. M.; Juutinen, S.; Julin, R.; Ketelhut, S.; Leino, M.; Nyman, M.; Rahkila, P.; Saren, J.; Scholey, C.

    2008-10-15

    Excited states of the extremely neutron-deficient nucleus {sup 197}At have been studied in an in-beam experiment using the fusion-evaporation reaction {sup 118}Sn({sup 82}Kr,p2n){sup 197}At. {gamma} rays belonging to {sup 197}At feeding the I{sup {pi}}=(9/2{sup -}) ground state, as well as {gamma} rays feeding the 311-keV I{sup {pi}}=(13/2{sup +}) isomer, decaying via the emission of {gamma} rays, and the 52-keV I{sup {pi}}=(1/2{sup +}){alpha}-decaying isomer have been identified using the recoil-{alpha}-decay tagging technique. Total Routhian surface calculations predict a near-spherical shape for the (9/2{sup -}) ground state and oblate shapes with {beta}{sub 2} around -0.2 for the (1/2{sup +}) and the (13/2{sup +}) states. These predictions agree with our experimental findings.

  15. Low-spin structure of 156Dy through gamma-ray spectroscopy

    SciTech Connect

    Caprio, M.A.; Zamfir, N.V.; Casten, R.F.; Barton, C.J.; Beausang, C.W.; Cooper, J.R.; Hecht, A.A.; Kruecken, R.; Newman, H.; Novak, J.R.; Pietralla, N.; Wolf, A.; Zyromski, K.E.

    2002-11-27

    Excited states of 156Dy were populated by beta decay and studied through gamma-ray spectroscopy. Extensive data led to improved information of the electromagnetic properties of low-spin states and to a substantially revised level scheme. The results are compared to those of other N=90 isotones and to predictions of the X(5) dynamical symmetry.

  16. Mass measurement of 80Y by beta-gamma coincidence spectroscopy

    SciTech Connect

    Barton, C.J.; Brenner, D.S.; Zamfir, N.V.; Caprio, M.A.; Aprahamian, A.; Wiescher, M.C.; Beausang, C.W.; Berant, Z.; Casten, R.F.; Cooper, J.R.; Gill, R.L.; Kruecken, R.; Novak, J.R.; Pietralla, N.; Shawcross, M.; Teymurazyan, A.; Wolf, A.

    2003-03-24

    The Qec value for 80Y has been measured by beta-gamma coincidence spectroscopy. Combining this result with the adopted mass excess of the daughter 80Sr gives a mass excess of >-61376(83) keV. Results are compared with other measurements and predictions of mass formulas. Implications of this measurement are considered for the rp-process.

  17. Development of Magnetic Microcalorimeters for Gamma-Ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Le, L. N.; Hummatov, R.; Hall, J. A.; Cantor, R. C.; Boyd, S. T. P.

    2016-01-01

    Integrating the SQUIDs and sensing coils of magnetic microcalorimeters onto the same die is a promising approach for maximizing flux coupling and signal/noise. However, new challenges in microfabrication must be overcome, because the underlying SQUID devices are sensitive to chemical attack and elevated processing temperatures. In this report, we describe development and details of a microfabrication process for integrated SQUID/sensor gamma-ray magnetic microcalorimeters with electroformed gold absorbers, starting from a modified version of the STAR Cryoelectronics "Delta 1000" Josephson Junction process.

  18. Gamma-ray spectroscopy: The diffuse galactic glow

    NASA Technical Reports Server (NTRS)

    Hartmann, Dieter H.

    1991-01-01

    The goal of this project is the development of a numerical code that provides statistical models of the sky distribution of gamma-ray lines due to the production of radioactive isotopes by ongoing Galactic nucleosynthesis. We are particularly interested in quasi-steady emission from novae, supernovae, and stellar winds, but continuum radiation and transient sources must also be considered. We have made significant progress during the first half period of this project and expect the timely completion of a code that can be applied to Oriented Scintillation Spectrometer Experiment (OSSE) Galactic plane survey data.

  19. Development of Magnetic Microcalorimeters for Gamma-Ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Le, L. N.; Hummatov, R.; Hall, J. A.; Cantor, R. C.; Boyd, S. T. P.

    2016-07-01

    Integrating the SQUIDs and sensing coils of magnetic microcalorimeters onto the same die is a promising approach for maximizing flux coupling and signal/noise. However, new challenges in microfabrication must be overcome, because the underlying SQUID devices are sensitive to chemical attack and elevated processing temperatures. In this report, we describe development and details of a microfabrication process for integrated SQUID/sensor gamma-ray magnetic microcalorimeters with electroformed gold absorbers, starting from a modified version of the STAR Cryoelectronics "Delta 1000" Josephson Junction process.

  20. Low background counting of 222Rn, 220Rn and 219Rn with electrostatic counters

    NASA Astrophysics Data System (ADS)

    Mong, Brian; EXO-200 Collaboration; nEXO Collaboration

    2014-09-01

    The radon counting technique based on electrostatic precipitation of progenies in gas followed by alpha spectroscopy has been applied to support the material selection programs of low background, neutrino and dark matter experiments with emphasis on EXO. An array of 8 counters operated by Laurentian University at SNOLAB and the Waste Isolation Pilot Plant have reached the sensitivity of 10 atoms/day in the uranium, thorium and actinium chains. Hardware improvements are underway to further increase the capacity and sensitivity in support of nEXO. The radon counting technique based on electrostatic precipitation of progenies in gas followed by alpha spectroscopy has been applied to support the material selection programs of low background, neutrino and dark matter experiments with emphasis on EXO. An array of 8 counters operated by Laurentian University at SNOLAB and the Waste Isolation Pilot Plant have reached the sensitivity of 10 atoms/day in the uranium, thorium and actinium chains. Hardware improvements are underway to further increase the capacity and sensitivity in support of nEXO. Supported by NSERC Project Grants ``Search for Double Beta Decay with EXO.''

  1. Environmental Radioactivity: Gamma Ray Spectroscopy with Germanium detector

    NASA Astrophysics Data System (ADS)

    Vyas, Gargi; Beausang, Cornelius; Hughes, Richard; Tarlow, Thomas; Gell, Kristen; University of Richmond Physics Team

    2013-10-01

    A CF-1000BRL series portable Air Particle Sampler with filter paper as filter media was placed in one indoor and one outdoor location at 100 LPM flow rate on six dates under alternating rainy and warm weather conditions over the course of sixteen days in May 2013. The machine running times spanned between 6 to 69 hours. Each filter paper was then put in a germanium gamma ray detector, and the counts ranged from 93000 to 250000 seconds. The spectra obtained were analyzed by the CANBERRA Genie 2000 software, corrected using a background spectrum, and calibrated using a 20.27 kBq activity multi-nuclide source. We graphed the corrected counts (from detector analysis time)/second (from air sampler running time)/liter (from the air sampler's flow rate) of sharp, significantly big peaks corresponding to a nuclide in every sample against the sample number along with error bars. The graphs were then used to compare the samples and they showed a similar trend. The slight differences were usually due to the different running times of the air sampler. The graphs of about 22 nuclides were analyzed. We also tried to recognize the nuclei to which several gamma rays belonged that were displayed but not recognized by the Genie 2000 software.

  2. Instructions for calibrating gamma detectors using the Canberra-Nuclear Data Genie Gamma Spectroscopy System

    SciTech Connect

    Brunk, J.L.

    1995-09-01

    A straight forward protocol provides a way to guide the calibration of a gamma detector for a particular geometry and material. Several programs have used the Low Level Gamma Counting Facility of the Health and Ecological Assessment Division of the Lawrence Livermore National Laboratory to count a variety of large environmental samples contained in several unique geometries. The equipment and calibration requirements needed to analyze these types of samples are explained. This document describes the calibration protocol that has been developed and describes how it is used to calibrate the detectors.

  3. HIGH ENERGY DELAYED GAMMA SPECTROSCOPY FOR PLUTONIUM ASSAY OF SPENT REACTOR FUEL

    SciTech Connect

    Campbell, Luke W.; Smith, L. E.; Misner, Alex C.

    2011-07-18

    Nuclear safeguards requires accountancy of plutonium present in spent reactor fuels. Current non-destructive methods do not directly measure plutonium content but instead rely on indirect measurements that require operator declarations of the fuel history. Delayed gamma spectroscopy is one method being investigated which can overcome these limitations. Delayed gamma rays from fission depend on the isotopic fission yield of the fissile isotope, and thus can be used to fingerprint the isotopes undergoing fission. However, difficulties arise because of the intense background due to long lived fission radionuclides already present in the fuel. We report on progress on simulated measurements of the delayed gamma spectrum in the presence of this background, using neutrons from a D-T source thermalized in an interrogation chamber slipped over a fuel assembly. By focusing on delayed gammas in the 3 to 4 MeV range, the passive spectrum becomes negligible, while allowing the preferential attenuation of the passive background to acceptable levels.

  4. Low-background tracker development for SuperNEMO

    SciTech Connect

    Mott, James; Collaboration: SuperNEMO Collaboration; and others

    2013-08-08

    The SuperNEMO experiment will search for neutrinoless double beta decay (0νββ) with a target sensitivity of T{sub 1/2}(0ν) > 10{sup 26} years, corresponding to an effective neutrino mass of 50-100 meV. At its heart there is a low-background gaseous tracking detector which allows for extremely efficient background rejection and, if 0νββ is observed, may provide important insights into the mechanism via which it may be mediated. Radon inside the tracker, which can mimic rare ββ events, is one of the most dangerous backgrounds for SuperNEMO. To reach the target sensitivity the radon concentration inside the tracking volume must be < 0.15 mBq/m{sup 3}. To reach this challengingly-low level of radon, a considerable program of R and D has been undertaken. This includes automation of the tracker-wiring process, development of a dedicated setup to measure radon diffusion and a 'radon concentration line' which will be able to measure levels of radon in the μBq/m{sup 3} range.

  5. Achieving low backgrounds in a variety of situations

    SciTech Connect

    Miley, H.S.; Brodzinski, R.L.; Reeves, J.H.; Avignone, F.T.

    1994-04-01

    To be sufficiently interesting, a physics experiment must measure a process that is relatively rare. The process may be rare due to small cross sections, low detector mass, or low detector efficiency. In any case, the process of interest must compete with processes in the detector`s environment that are much more prolific. Although these processes may have been of interest last year, they serve only to hide signals of interest today. The most common method of background reduction is to construct a lead shield around the detector. A less common technique is to reconstruct a detector apparatus with materials with a lower specific activity. The effects of cosmic rays are also frequently reduced by using an active veto system or relocating underground. However, the judicious use of these and other techniques requires some knowledge of the vulnerability of the detector and the relative sizes of potential backgrounds. The Pacific Northwest Laboratory-University of South Carolina (PNL-USC) double beta-decay collaboration and more recently the International Germanium Experiment (IGEX) collaboration have accrued a great deal of experience with semiconductor detectors operated above ground, in shallow below-ground locations (36 m), and in several deep underground locations. The effect of low-background materials, coincidence techniques, cosmic neutrons, and ubiquitous uranium and thorium decay products will be discussed as a function of depth and specifically for above-ground experiments.

  6. Measurement techniques for characterizing and using low background germanium detectors

    NASA Astrophysics Data System (ADS)

    Zimmer, William H.; Wagner, Sanford E.

    1984-06-01

    An investigation has been undertaken to determine whether an order of magnitude background reduction from present typical cryostat-detector systems can be obtained through the use of low background components. In order to measure progress in this task, a standard, ten-centimeter lead shield was fitted with a five-centimeter, oxygen-free high-conductivity copper liner and a borated polyethylene neutron absorber. This reduced the contribution of uranium-238, thorium daughters, and radium daughters from the shield as seen by the detector by 1.3, 0.02, and 0.1 Bq respectively. The methodology of determining very low net photon peak areas in the presence of high continuum levels to assure maximum accuracy was verified and is presented. By these means the background activities of detectors are being measured at the -10 2 Bq per nuclide and detector component materials at the Bq per gram level, both with total uncertainties of less than 50% 1σ. The hardware and software developed is being used to measure the background activity of the detectors and for the analysis of low activity samples.

  7. High resolution spectroscopy from low altitude satellites. [gamma ray astronomy

    NASA Technical Reports Server (NTRS)

    Nakano, G. H.; Imhof, W. L.

    1978-01-01

    The P 78 1 satellite to be placed in a synchronous polar orbit at an altitude of 550-660 km will carry two identical high resolution spectrometers each consisting of a single (approximately 85 cc) intrinsic germanium IGE detector. The payload also includes a pair of phoswitch scintillators, an array of CdTe detectors and several particle detectors, all of which are mounted on the wheel of the satellite. The intrinsic high purity IGE detectors receive cooling from two Stirling cycle refrigerators and facilitate the assembly of large and complex detector arrays planned for the next generation of high sensitivity instruments such as those planned for the gamma ray observatory. The major subsystems of the spectrometer are discussed as well as its capabilities.

  8. Isotopically enriched germanium detectors for astrophysical gamma-ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Gehrels, Neil

    1990-01-01

    A study is presented of the instrumental background in astrophysical gamma-ray spectrometers using isotopically enriched germanium detectors. Calculations show that the beta-decay background, which is the largest component between approximately 0.1 and 1.0 MeV in balloonborne and satellite spectrometers, is dominated by the activation of Ge-74. This component can be reduced by an order of magnitude using detectors enriched to more than 80 percent in (Ge-70). The predicted reduction in the total background for current balloonborne instruments is more than a factor of 1.7 between 0.2 and 1.0 MeV. For future satellite instruments, the reduction in this energy range is by more than a factor of 5.

  9. In-beam gamma-ray spectroscopy at the RIBF

    SciTech Connect

    Doornenbal, Pieter

    2015-10-15

    At the Radioactive Isotope Beam Factory stable primary beams are accelerated up to 345 MeV/u and incident on a primary target to produce secondary cocktail beams with the fragment separator BigRIPS ranging from the lightest nuclei up to the uranium region. For in-beam γ-ray spectroscopy, the secondary beam impinge on a reaction target at energies between 100 and 300 MeV/u. Reaction residues are identified with the ZeroDegree spectrometer and γ-rays detected with the NaI(Tl) based DALI2 array. This conference paper outlines the experimental setup and presents recent exemplary results.

  10. Study well-shaped germanium detectors for low-background counting

    NASA Astrophysics Data System (ADS)

    Wei, W.-Z.; Mei, D.-M.; Zhang, C.

    2015-05-01

    Radiogenic particles are known as the main sources of background for all ultra-low background experiments in the detection of dark matter and neutrino properties. In particular, the radiogenic gamma rays from PMTs are a main component of the observed backgrounds in the noble liquid detectors such as XENON100 and LUX. This suggests a more accurate screening of PMTs is needed for the next generation experiments such as LUX-Zplin or Xenon1T. Hence, we propose to develop well-shaped germanium detectors for a better understanding of the radiogenic background from PMTs. A well-shaped germanium detector array and PMT (R11410MOD) have been designed in a Geant4-based Monte Carlo simulation, in which three radiogenic background isotopes from 238U, 232Th and 40K have been studied. In this work, we show the detector performance including the detector efficiency, energy resolution and the detector sensitivity for low-background counting in the detection of rare event physics.

  11. Calibration of an Ultra-Low-Background Proportional Counter for Measuring 37Ar

    SciTech Connect

    Seifert, Allen; Aalseth, Craig E.; Bonicalzi, Ricco; Bowyer, Ted W.; Day, Anthony R.; Fuller, Erin S.; Haas, Derek A.; Hayes, James C.; Hoppe, Eric W.; Humble, Paul H.; Keillor, Martin E.; LaFerriere, Brian D.; Mace, Emily K.; McIntyre, Justin I.; Merriman, Jason H.; Miley, Harry S.; Myers, Allan W.; Orrell, John L.; Overman, Cory T.; Panisko, Mark E.; Williams, Richard M.

    2013-08-08

    Abstract. An ultra-low-background proportional counter (ULBPC) design has been developed at Pacific Northwest National Laboratory (PNNL) using clean materials, primarily electrochemically-purified copper. This detector, along with an ultra-low-background counting system (ULBCS), was developed to complement a new shallow underground laboratory (30 meters water-equivalent) constructed at PNNL. The ULBCS design includes passive neutron and gamma shielding, along with an active cosmic-veto system. This system provides a capability for making ultra-sensitive measurements to support applications like age-dating soil hydrocarbons with 14C/3H, age-dating of groundwater with 39Ar, and soil-gas assay for 37Ar to support On-Site Inspection (OSI). On-Site Inspection is a key component of the verification regime for the Comprehensive Nuclear-Test-Ban Treaty (CTBT). Measurements of radionuclides created by an underground nuclear explosion are valuable signatures of a Treaty violation. For OSI, the 35-day half-life of 37Ar, produced from neutron interactions with calcium in soil, provides both high specific activity and sufficient time for inspection before decay limits sensitivity. This work describes the calibration techniques and analysis methods developed to enable quantitative measurements of 37Ar samples over a broad range of pressures. These efforts, along with parallel work in progress on gas chemistry separation, are expected to provide a significant new capability for 37Ar soil gas background studies.

  12. Calibration of an ultra-low-background proportional counter for measuring {sup 37}Ar

    SciTech Connect

    Seifert, A.; Aalseth, C. E.; Bonicalzi, R. M.; Bowyer, T. W.; Day, A. R.; Fuller, E. S.; Haas, D. A.; Hayes, J. C.; Hoppe, E. W.; Humble, P. H.; Keillor, M. E.; LaFerriere, B. D.; Mace, E. K.; McIntyre, J. I.; Merriman, J. H.; Miley, H. S.; Myers, A. W.; Orrell, J. L.; Overman, C. T.; Panisko, M. E.; and others

    2013-08-08

    An ultra-low-background proportional counter design has been developed at Pacific Northwest National Laboratory (PNNL) using clean materials, primarily electro-chemically-purified copper. This detector, along with an ultra-low-background counting system (ULBCS), was developed to complement a new shallow underground laboratory (30 meters water-equivalent) at PNNL. The ULBCS design includes passive neutron and gamma shielding, along with an active cosmic-veto system. This system provides a capability for making ultra-sensitive measurements to support applications like age-dating soil hydrocarbons with {sup 14}C/{sup 3}H, age-dating of groundwater with {sup 39}Ar, and soil-gas assay for {sup 37}Ar to support On-Site Inspection (OSI). On-Site Inspection is a key component of the verification regime for the Comprehensive Nuclear-Test-Ban Treaty (CTBT). Measurements of radionuclides created by an underground nuclear explosion are valuable signatures of a Treaty violation. For OSI, the 35-day half-life of {sup 37}Ar, produced from neutron interactions with calcium in soil, provides both high specific activity and sufficient time for inspection before decay limits sensitivity. This work describes the calibration techniques and analysis methods developed to enable quantitative measurements of {sup 37}Ar samples over a broad range of proportional counter operating pressures. These efforts, along with parallel work in progress on gas chemistry separation, are expected to provide a significant new capability for {sup 37}Ar soil gas background studies.

  13. Sensitivity of LDEF foil analyses using ultra-low background germanium vs. large NaI(Tl) multidimensional spectrometers

    NASA Technical Reports Server (NTRS)

    Reeves, James H.; Arthur, Richard J.; Brodzinski, Ronald L.

    1993-01-01

    Cobalt foils and stainless steel samples were analyzed for induced Co-60 activity with both an ultra-low background germanium gamma-ray spectrometer and with a large NaI(Tl) multidimensional spectrometer, both of which use electronic anticoincidence shielding to reduce background counts resulting from cosmic rays. Aluminum samples were analyzed for Na-22. The results, in addition to the relative sensitivities and precisions afforded by the two methods, are presented.

  14. Low background high efficiency radiocesium detection system based on positron emission tomography technology

    SciTech Connect

    Yamamoto, Seiichi; Ogata, Yoshimune

    2013-09-15

    After the 2011 nuclear power plant accident at Fukushima, radiocesium contamination in food became a serious concern in Japan. However, low background and high efficiency radiocesium detectors are expensive and huge, including semiconductor germanium detectors. To solve this problem, we developed a radiocesium detector by employing positron emission tomography (PET) technology. Because {sup 134}Cs emits two gamma photons (795 and 605 keV) within 5 ps, they can selectively be measured with coincidence. Such major environmental gamma photons as {sup 40}K (1.46 MeV) are single photon emitters and a coincidence measurement reduces the detection limit of radiocesium detectors. We arranged eight sets of Bi{sub 4}Ge{sub 3}O{sub 12} (BGO) scintillation detectors in double rings (four for each ring) and measured the coincidence between these detectors using PET data acquisition system. A 50 × 50 × 30 mm BGO was optically coupled to a 2 in. square photomultiplier tube (PMT). By measuring the coincidence, we eliminated most single gamma photons from the energy distribution and only detected those from {sup 134}Cs at an average efficiency of 12%. The minimum detectable concentration of the system for the 100 s acquisition time is less than half of the food monitor requirements in Japan (25 Bq/kg). These results show that the developed radiocesium detector based on PET technology is promising to detect low level radiocesium.

  15. Low background high efficiency radiocesium detection system based on positron emission tomography technology.

    PubMed

    Yamamoto, Seiichi; Ogata, Yoshimune

    2013-09-01

    After the 2011 nuclear power plant accident at Fukushima, radiocesium contamination in food became a serious concern in Japan. However, low background and high efficiency radiocesium detectors are expensive and huge, including semiconductor germanium detectors. To solve this problem, we developed a radiocesium detector by employing positron emission tomography (PET) technology. Because (134)Cs emits two gamma photons (795 and 605 keV) within 5 ps, they can selectively be measured with coincidence. Such major environmental gamma photons as (40)K (1.46 MeV) are single photon emitters and a coincidence measurement reduces the detection limit of radiocesium detectors. We arranged eight sets of Bi4Ge3O12 (BGO) scintillation detectors in double rings (four for each ring) and measured the coincidence between these detectors using PET data acquisition system. A 50 × 50 × 30 mm BGO was optically coupled to a 2 in. square photomultiplier tube (PMT). By measuring the coincidence, we eliminated most single gamma photons from the energy distribution and only detected those from (134)Cs at an average efficiency of 12%. The minimum detectable concentration of the system for the 100 s acquisition time is less than half of the food monitor requirements in Japan (25 Bq/kg). These results show that the developed radiocesium detector based on PET technology is promising to detect low level radiocesium. PMID:24089828

  16. Low background high efficiency radiocesium detection system based on positron emission tomography technology

    NASA Astrophysics Data System (ADS)

    Yamamoto, Seiichi; Ogata, Yoshimune

    2013-09-01

    After the 2011 nuclear power plant accident at Fukushima, radiocesium contamination in food became a serious concern in Japan. However, low background and high efficiency radiocesium detectors are expensive and huge, including semiconductor germanium detectors. To solve this problem, we developed a radiocesium detector by employing positron emission tomography (PET) technology. Because 134Cs emits two gamma photons (795 and 605 keV) within 5 ps, they can selectively be measured with coincidence. Such major environmental gamma photons as 40K (1.46 MeV) are single photon emitters and a coincidence measurement reduces the detection limit of radiocesium detectors. We arranged eight sets of Bi4Ge3O12 (BGO) scintillation detectors in double rings (four for each ring) and measured the coincidence between these detectors using PET data acquisition system. A 50 × 50 × 30 mm BGO was optically coupled to a 2 in. square photomultiplier tube (PMT). By measuring the coincidence, we eliminated most single gamma photons from the energy distribution and only detected those from 134Cs at an average efficiency of 12%. The minimum detectable concentration of the system for the 100 s acquisition time is less than half of the food monitor requirements in Japan (25 Bq/kg). These results show that the developed radiocesium detector based on PET technology is promising to detect low level radiocesium.

  17. A Shallow Underground Laboratory for Low-Background Radiation Measurements and Materials Development

    SciTech Connect

    Aalseth, Craig E.; Bonicalzi, Ricco; Cantaloub, Michael G.; Day, Anthony R.; Erikson, Luke E.; Fast, James E.; Forrester, Joel B.; Fuller, Erin S.; Glasgow, Brian D.; Greenwood, Lawrence R.; Hoppe, Eric W.; Hossbach, Todd W.; Hyronimus, Brian J.; Keillor, Martin E.; Mace, Emily K.; McIntyre, Justin I.; Merriman, Jason H.; Myers, Allan W.; Overman, Cory T.; Overman, Nicole R.; Panisko, Mark E.; Seifert, Allen; Warren, Glen A.; Runkle, Robert C.

    2012-11-08

    Abstract: Pacific Northwest National Laboratory recently commissioned a new shallow underground laboratory, located at a depth of approximately 30 meters water-equivalent. This new addition to the small class of radiation measurement laboratories located at modest underground depths worldwide houses the latest generation of custom-made, high-efficiency, low-background gamma-ray spectrometers and gas proportional counters. This manuscript describes the unique capabilities present in the shallow underground laboratory; these include large-scale ultra-pure materials production and a suite of radiation detection systems. Reported data characterize the degree of background reduction achieved through a combination of underground location, graded shielding, and rejection of cosmic-ray events. We conclude by presenting measurement targets and future opportunities.

  18. A shallow underground laboratory for low-background radiation measurements and materials development

    SciTech Connect

    Aalseth, C. E.; Bonicalzi, R. M.; Cantaloub, M. G.; Day, A. R.; Erikson, L. E.; Fast, J.; Forrester, J. B.; Fuller, E. S.; Glasgow, B. D.; Greenwood, L. R.; Hoppe, E. W.; Hossbach, T. W.; Hyronimus, B. J.; Keillor, M. E.; Mace, E. K.; McIntyre, J. I.; Merriman, J. H.; Myers, A. W.; Overman, C. T.; Overman, N. R.; and others

    2012-11-15

    Pacific Northwest National Laboratory recently commissioned a new shallow underground laboratory, located at a depth of approximately 30 meters-water-equivalent. This new addition to the small class of radiation measurement laboratories located at modest underground depths houses the latest generation of custom-made, high-efficiency, low-background gamma-ray spectrometers and gas proportional counters. This paper describes the unique capabilities present in the shallow underground laboratory; these include large-scale ultra-pure materials production and a suite of radiation detection systems. Reported data characterize the degree of background reduction achieved through a combination of underground location, graded shielding, and rejection of cosmic-ray events. We conclude by presenting measurement targets and future opportunities.

  19. A shallow underground laboratory for low-background radiation measurements and materials development

    NASA Astrophysics Data System (ADS)

    Aalseth, C. E.; Bonicalzi, R. M.; Cantaloub, M. G.; Day, A. R.; Erikson, L. E.; Fast, J.; Forrester, J. B.; Fuller, E. S.; Glasgow, B. D.; Greenwood, L. R.; Hoppe, E. W.; Hossbach, T. W.; Hyronimus, B. J.; Keillor, M. E.; Mace, E. K.; McIntyre, J. I.; Merriman, J. H.; Myers, A. W.; Overman, C. T.; Overman, N. R.; Panisko, M. E.; Seifert, A.; Warren, G. A.; Runkle, R. C.

    2012-11-01

    Pacific Northwest National Laboratory recently commissioned a new shallow underground laboratory, located at a depth of approximately 30 meters-water-equivalent. This new addition to the small class of radiation measurement laboratories located at modest underground depths houses the latest generation of custom-made, high-efficiency, low-background gamma-ray spectrometers and gas proportional counters. This paper describes the unique capabilities present in the shallow underground laboratory; these include large-scale ultra-pure materials production and a suite of radiation detection systems. Reported data characterize the degree of background reduction achieved through a combination of underground location, graded shielding, and rejection of cosmic-ray events. We conclude by presenting measurement targets and future opportunities.

  20. A broadband THz receiver for low background space applications

    NASA Astrophysics Data System (ADS)

    Hagmann, C.; Benford, D. J.; Clapp, A. C.; Richards, P. L.; Timbie, P.

    We have developed a sensitive bolometric receiver for low background space applications. In a 10 percent bandwidth at 1 THz, this receiver is approximately 100 times more sensitive than a quantum limited heterodyne receiver with a 1 GHz IF bandwidth. This receiver is designed to be used for the long wavelength band (200-700 microns) in the MIPS instrument on NASA's SIRTF satellite. The bolometers are cooled to 100 mK by an adiabatic demagnetization refrigerator. Roughly 60 g of cesium chrome alum salt is partially demagnetized to 100 mK, followed by a slow regulated downramp to compensate for the heat leak. The hold time of the ADR system is about 18 hours with a temperature stability of delta T(sub rms) approx. equals 10 micro-K. The composite bolometers have electrical responsivities of 10(exp 9)V/W and electrical NEP's of about 3x10(exp -17) W/square root of Hz. The bolometer signals are read out by JFET preamplifiers located on the helium plate and operated at 120 K. We have addressed a number of space qualification issues, such as the development of an analog magnet controller, construction of a cryogenic shake-table for bolometers and selection of the paramagnetic salt CCA which can survive a bakeout at 50 C. The receiver is scheduled to be flown in the spring of 1992 on a balloon telescope. This flight has a dual purpose. One is to provide realistic test of the capabilities of the new receiver. The other is to search for anisotropies in the cosmic microwave background on scales of a few degrees.

  1. A broadband THz receiver for low background space applications

    NASA Technical Reports Server (NTRS)

    Hagmann, C.; Benford, D. J.; Clapp, A. C.; Richards, P. L.; Timbie, P.

    1992-01-01

    We have developed a sensitive bolometric receiver for low background space applications. In a 10 percent bandwidth at 1 THz, this receiver is approximately 100 times more sensitive than a quantum limited heterodyne receiver with a 1 GHz IF bandwidth. This receiver is designed to be used for the long wavelength band (200-700 microns) in the MIPS instrument on NASA's SIRTF satellite. The bolometers are cooled to 100 mK by an adiabatic demagnetization refrigerator. Roughly 60 g of cesium chrome alum salt is partially demagnetized to 100 mK, followed by a slow regulated downramp to compensate for the heat leak. The hold time of the ADR system is about 18 hours with a temperature stability of delta T(sub rms) approx. equals 10 micro-K. The composite bolometers have electrical responsivities of 10(exp 9)V/W and electrical NEP's of about 3x10(exp -17) W/square root of Hz. The bolometer signals are read out by JFET preamplifiers located on the helium plate and operated at 120 K. We have addressed a number of space qualification issues, such as the development of an analog magnet controller, construction of a cryogenic shake-table for bolometers and selection of the paramagnetic salt CCA which can survive a bakeout at 50 C. The receiver is scheduled to be flown in the spring of 1992 on a balloon telescope. This flight has a dual purpose. One is to provide realistic test of the capabilities of the new receiver. The other is to search for anisotropies in the cosmic microwave background on scales of a few degrees.

  2. Electrochemical impedance spectroscopy based-on interferon-gamma detection

    NASA Astrophysics Data System (ADS)

    Li, Guan-Wei; Kuo, Yi-Ching; Tsai, Pei-I.; Lee, Chih-Kung

    2014-03-01

    Tuberculosis (TB) is an ancient disease constituted a long-term menace to public health. According to World Health Organization (WHO), mycobacterium tuberculosis (MTB) infected nearly a third of people of the world. There is about one new TB occurrence every second. Interferon-gamma (IFN-γ) is associated with susceptibility to TB, and interferongamma release assays (IGRA) is considered to be the best alternative of tuberculin skin test (TST) for diagnosis of latent tuberculosis infection (LTBI). Although significant progress has been made with regard to the design of enzyme immunoassays for IFN-γ, adopting this assay is still labor-intensive and time-consuming. To alleviate these drawbacks, we used IFN-γ antibody to facilitate the detection of IFN-γ. An experimental verification on the performance of IGRA was done in this research. We developed two biosensor configurations, both of which possess high sensitivity, specificity, and rapid IFN-γ diagnoses. The first is the electrochemical method. The second is a circular polarization interferometry configuration, which incorporates two light beams with p-polarization and s-polarization states individually along a common path, a four photo-detector quadrature configuration to arrive at a phase modulated ellipsometer. With these two methods, interaction between IFN-γ antibody and IFN-γ were explored and presented in detail.

  3. Identification of gamma-irradiated fruit juices by EPR spectroscopy

    NASA Astrophysics Data System (ADS)

    Aleksieva, K. I.; Dimov, K. G.; Yordanov, N. D.

    2014-10-01

    The results of electron paramagnetic resonance (EPR) study on commercially available juices from various fruits and different fruit contents: 25%, 40%, 50%, and 100%, homemade juices, nectars and concentrated fruit syrups, before and after gamma-irradiation are reported. In order to remove water from non- and irradiated samples all juices and nectars were filtered; the solid residue was washed with alcohol and dried at room temperature. Only concentrated fruit syrups were dried for 60 min at 40 °C in a standard laboratory oven. All samples under study show a singlet EPR line with g=2.0025 before irradiation with exception of concentrated fruit syrups, which are EPR silent. Irradiation of juice samples gives rise to complex EPR spectra which gradually transferred to “cellulose-like” EPR spectrum from 25% to 100% fruit content. Concentrated fruit syrups show typical “sugar-like“ spectra due to added saccharides. All EPR spectra are characteristic and can prove radiation treatment. The fading kinetics of radiation-induced EPR signals were studied for a period of 60 days after irradiation.

  4. SrI2 scintillator for gamma ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Cherepy, N. J.; Sturm, B. W.; Drury, O. B.; Hurst, T. A.; Sheets, S. A.; Ahle, L. E.; Saw, C. K.; Pearson, M. A.; Payne, S. A.; Burger, A.; Boatner, L. A.; Ramey, J. O.; van Loef, E. V.; Glodo, J.; Hawrami, R.; Higgins, W. M.; Shah, K. S.; Moses, W. W.

    2009-08-01

    We are working to perfect the growth of divalent Eu-doped strontium iodide single crystals and to optimize the design of SrI2(Eu)-based gamma ray spectrometers. SrI2(Eu) offers a light yield in excess of 100,000 photons/MeV and light yield proportionality surpassing that of Ce-doped lanthanum bromide. Thermal and x-ray diffraction analyses of SrI2 and EuI2 indicate an excellent match in melting and crystallographic parameters, and very modest thermal expansion anisotropy. We have demonstrated energy resolution with SrI2(4-6%Eu) of 2.6% at 662 keV and 7.6% at 60 keV with small crystals, while the resolution degrades somewhat for larger sizes. Our experiments suggest that digital techniques may be useful in improving the energy resolution in large crystals impaired by light-trapping, in which scintillation light is re-absorbed and re-emitted in large and/or highly Eu2+ -doped crystals. The light yield proportionality of SrI2(Eu) is found to be superior to that of other known scintillator materials, such as LaBr3(Ce) and NaI(Tl).

  5. A silicon photomultiplier readout for time of flight neutron spectroscopy with {gamma}-ray detectors

    SciTech Connect

    Pietropaolo, A.; Gorini, G.; Festa, G.; Andreani, C.; De Pascale, M. P.; Reali, E.; Grazzi, F.; Schooneveld, E. M.

    2009-09-15

    The silicon photomultiplier (SiPM) is a recently developed photosensor used in particle physics, e.g., for detection of minimum ionizing particles and/or Cherenkov radiation. Its performance is comparable to that of photomultiplier tubes, but with advantages in terms of reduced volume and magnetic field insensitivity. In the present study, the performance of a gamma ray detector made of an yttrium aluminum perovskite scintillation crystal and a SiPM-based readout is assessed for use in time of flight neutron spectroscopy. Measurements performed at the ISIS pulsed neutron source demonstrate the feasibility of {gamma}-detection based on the new device.

  6. Neutron-induced gamma-ray spectroscopy: simulations for chemical mapping of planetary surfaces

    SciTech Connect

    Brueckner, J.; Waenke, H.; Reedy, R.C.

    1986-01-01

    Cosmic rays interact with the surface of a planetary body and produce a cascade of secondary particles, such as neutrons. Neutron-induced scattering and capture reactions play an important role in the production of discrete gamma-ray lines that can be measured by a gamma-ray spectrometer on board of an orbiting spacecraft. These data can be used to determine the concentration of many elements in the surface of a planetary body, which provides clues to its bulk composition and in turn to its origin and evolution. To investigate the gamma rays made by neutron interactions, thin targets were irradiated with neutrons having energies from 14 MeV to 0.025 eV. By means of foil activation technique the ratio of epithermal to thermal neutrons was determined to be similar to that in the Moon. Gamma rays emitted by the targets and the surrounding material were detected by a high-resolution germanium detector in the energy range of 0.1 to 8 MeV. Most of the gamma-ray lines that are expected to be used for planetary gamma-ray spectroscopy were found in the recorded spectra and the principal lines in these spectra are presented. 58 refs., 7 figs., 9 tabs.

  7. Gamma-ray and neutron spectroscopy of planetary surfaces and atmospheres

    SciTech Connect

    Reedy, R.C.

    1987-01-01

    The neutrons and gamma rays escaping from a planet can be used to map the concentrations of various elements in its surface. In a planet, the high-energy particles in the galactic cosmic rays induce a cascade of particles that includes many neutrons. The ..gamma.. rays are made by the decay of the naturally-occurring radioelements and by nuclear excitations induced by cosmic-ray particles and their secondaries (especially neutron capture or inelastic scattering reactions). After a short history of planetary ..gamma..-ray and neutron spectroscopy, the ..gamma..-ray spectrometer and active neutron detection system planned for the Mars Observer Mission are presented. The results of laboratory experiments that simulate the cosmic-ray bombardments of planetary surfaces and the status of the theoretical calculations for the processes that make and transport neutrons and ..gamma.. rays will be reviewed. Studies of Mars, including its atmosphere, are emphasized, as are new ideas, concepts, and problems that have arisen over the last decade, such as Doppler broadening and peaks from neutron scattering with germanium nuclei in a ..gamma..-ray spectrometer. 23 refs., 1 fig.

  8. Towards combining in-beam {gamma}-ray and conversion electron spectroscopy

    SciTech Connect

    Papadakis, P.; Herzberg, R.-D.; Pakarinen, J.; Butler, P. A.; Cresswell, J. R.; Page, R. D.; Parr, E.; Seddon, D. A.; Thornhill, J.; Wells, D.; Coleman-Smith, P. J.; Lazarus, I. H.; Letts, S. C.; Pucknell, V. F. E.; Simpson, J.; Greenlees, P. T.; Jones, P.; Julin, R.; Peura, P.; Rahkila, P.

    2009-01-28

    The SAGE spectrometer will combine a segmented Si-detector with a Ge-detector array aiming to take the simultaneous in-beam {gamma}-ray and conversion electron spectroscopy to the next level. It will be coupled with the GREAT focal plane spectrometer and the RITU gas-filled recoil separator at the accelerator laboratory of the University of Jyvaeskylae, Finland. Its high efficiency and resolution will open the door to a new era of complete spectroscopy directed, amongst others, at the study of superheavy nuclei aiming to investigate the properties of the next spherical proton shell above Z = 82.

  9. Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

    SciTech Connect

    Ludewigt, Bernhard; Mozin, Vladimir; Campbell, Luke; Favalli, Andrea; Alan W. Hunt; Edward T. Reedy; Heather A. Seipel

    2015-06-01

    Modeling capabilities were added to an existing framework and codes were adapted as needed for analyzing experiments and assessing application-specific assay concepts including simulation of measurements over many short irradiation/spectroscopy cycles. The code package was benchmarked against the data collected at the IAC for small targets and assembly-scale data collected at LANL. A study of delayed gamma-ray spectroscopy for nuclear safeguards was performed for a variety of assemblies in the extensive NGSI spent fuel library. The modeling results indicate that delayed gamma-ray responses can be collected from spent fuel assemblies with statistical quality sufficient for analyzing their isotopic composition using a 1011 n/s neutron generator and COTS detector instrumentation.

  10. Germanium-Based Detectors for Gamma-Ray Imaging andSpectroscopy

    SciTech Connect

    Amman, Mark; Luke, Paul N.; Boggs, Steven E.

    2006-10-13

    Germanium-based detectors are the standard technology usedfor gamma-ray spectroscopy when high efficiency and excellent energyresolution are desired. By dividing the electrical contacts on thesedetectors into segments, the locations of the gamma-ray interactionevents within the detectors can be determined as well as the depositedenergies. This enables simultaneous gamma-ray imaging and spectroscopyand leads to applications in the areas of astronomy, nuclear physics,environmental remediation, nuclear nonproliferation, and homelandsecurity. Producing the fine-pitched electrode segmentation oftenrequired for imaging has been problematic in the past. To address thisissue, we have developed an amorphous-semiconductor contact technology.Using this technology, fully passivated detectors with closely spacedcontacts can be produced using a simple fabrication process. The currentstate of the amorphous-semiconductor contact technology and thechallenges that remain will be given in this paper.

  11. X-ray and. gamma. -ray spectroscopy of solids under pressure

    SciTech Connect

    Ingalls, R.L.

    1990-04-20

    This report briefly describes our studies of various materials at high pressures by means of x-ray and {gamma}-ray absorption spectroscopy. High pressure provides a very effective means of studying materials. Virtually every property is altered from the color and crystal structure to the electrical and magnetic properties. The fundamental reason, of course, is that the quantum levels depend upon the atomic spacing so that both the electronic and vibrational structure is affected.

  12. {gamma}-Spectroscopy of Positive Parity Bands In The {sup 156}Gd Nucleus

    SciTech Connect

    Vancraeyenest, A.; Guinet, D.; Stezowski, O.; Doan, Q. T.; Redon, N.; Greenlees, P. T.; Jones, P.

    2011-10-28

    During an experiment at Jyvaeskylae laboratory involving a 27 MeV {alpha} beam on a thick {sup 154}Sm target, {gamma}-spectroscopy of {sup 156}Gd was performed using JUROGAM HPGe multidetector array. We will present here experimental results concerning positive parity bands of this nucleus. Level scheme was enriched with more than ten new transitions as well as a new level in a band observed recently.

  13. Ge-diode detector combined with crystal-diffraction spectrometer permits high-resolution gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Namenson, A. I.; Smither, R. K.

    1969-01-01

    Crystal-diffraction spectrometer, combined with a lithium-drifted Ge-diode detector, performs high-resolution gamma ray spectroscopy on the complicated neutron-capture gamma ray spectra. The system is most useful in the 1-3 MeV energy range and improves the signal to background ratio.

  14. The transient gamma-ray spectrometer: A new high resolution detector for gamma-ray burst spectroscopy

    SciTech Connect

    Seifert, H.; Baker, R.; Cline, T.L.; Gehrels, N.; Jermakian, J.; Nolan, T.; Ramaty, R.; Sheppard, D.A.; Smith, G.; Stilwell, D.E.; Teegarden, B.J.; Trombka, J.; Owens, A.; Cork, C.P.; Landis, D.A.; Luke, P.N.; Madden, N.W.; Malone, D.; Pehl, R.H.; Yaver, H.; Hurley, K.; Mathias, S.; Post, A.H. Jr.

    1992-01-01

    The Transient Gamma-Ray Spectrometer (TGRS) to be flown aboard the WIND spacecraft is primarily designed to perform high resolution spectroscopy of transient gamma-ray events, such as cosmic [gamma]-ray bursts and solar flares, over the energy range 20 keV to 10 MeV with an expected spectroscopic resolution of E/[delta]E = 500. The detector itself consists of a 215 cm[sup 3] high purity n-type Ge crystal kept at cryogenic temperatures by a passive radiative cooler. The geometric field of view defined by the cooler is 170[degrees]. To avoid continuous triggers caused by soft solar events, a thin Be/Cu sun-shield around the sides of the cooler has been provided. A passive Mo/Pb occulter, which modulates signals from within [+-]5[degrees] of the ecliptic plane at the spacecraft spin frequency, is used to identify and study solar flares, as well as emission from the galactic plane and center. Thus, in addition to transient event measurements, the instrument will allow the search for possible diffuse background lines and monitor the 511 keV positron annihilation radiation from the galactic center. In order to handle the typically large burst count rates which can be in excess of 100 kHz, burst data are stored directly in an on-board 2.75 Mbit burst memory with an absolute timing accuracy of [+-]1.5 ms after ground processing. This capacity is sufficient to store the entire spectral data set of all but the largest bursts. The experiment is scheduled to be launched on a Delta II launch vehicle from Cape Canaveral in the fall of 1993.

  15. Monitoring of the interconversion of gamma-butyrolactone (GBL) to gamma hydroxybutyric acid (GHB) by Raman spectroscopy.

    PubMed

    Munshi, Tasnim; Brewster, Victoria L; Edwards, Howell G M; Hargreaves, Michael D; Jilani, Shelina K; Scowen, Ian J

    2013-08-01

    Gamma-hydroxybutyric acid (GHB) is a drug-of-abuse that has recently become associated with drug-facilitated sexual assault, known as date rape. For this reason the drug is commonly found 'spiked' in alcoholic beverages. When GHB is in solution it may undergo conversion into the corresponding lactone, Gamma-butyrolactone (GBL). Studies have been carried out to determine the detection limits of GHB and GBL in various solutions by Raman spectroscopy and to monitor the interconversion of GHB and GBL in solution with different pH conditions and temperature. In this study, a portable Raman spectrometer was used to study the interconversion of GHB and GBL in water and ethanol solutions as a function of pH, time, and temperature. The aim of this was to determine the optimum pH range for conversion in order to relate this to the pH ranges that the drug is likely to be subjected to, first in spiked beverages and secondly after ingestion in the digestive system. The aim was also to identify a timescale for this conversion in relation to possible scenarios, for example if GHB takes a number of hours to convert to GBL, it is likely for the beverage to be ingested before esterification can take place. GHB and GBL were then spiked into a selection of beverages of known pH in order to study the stability of GHB and GBL in real systems. PMID:23225646

  16. Exploitation of Geometric Occlusion and Covariance Spectroscopy in a Gamma Sensor Array

    SciTech Connect

    Mukhopadhyay, Sanjoy; Maurer, Richard; Wolff, Ronald; Mitchell, Stephen; Guss, Paul; Trainham, Clifford

    2013-09-01

    The National Security Technologies, LLC, Remote Sensing Laboratory has recently used an array of six small-footprint (1-inch diameter by 3-inch long) cylindrical crystals of thallium-doped sodium iodide scintillators to obtain angular information from discrete gamma ray–emitting point sources. Obtaining angular information in a near-field measurement for a field-deployed gamma sensor is a requirement for radiological emergency work. Three of the sensors sit at the vertices of a 2-inch isosceles triangle, while the other three sit on the circumference of a 3-inch-radius circle centered in this triangle. This configuration exploits occlusion of sensors, correlation from Compton scattering within a detector array, and covariance spectroscopy, a spectral coincidence technique. Careful placement and orientation of individual detectors with reference to other detectors in an array can provide improved angular resolution for determining the source position by occlusion mechanism. By evaluating the values of, and the uncertainties in, the photopeak areas, efficiencies, branching ratio, peak area correction factors, and the correlations between these quantities, one can determine the precise activity of a particular radioisotope from a mixture of radioisotopes that have overlapping photopeaks that are ordinarily hard to deconvolve. The spectral coincidence technique, often known as covariance spectroscopy, examines the correlations and fluctuations in data that contain valuable information about radiation sources, transport media, and detection systems. Covariance spectroscopy enhances radionuclide identification techniques, provides directional information, and makes weaker gamma-ray emission—normally undetectable by common spectroscopic analysis—detectable. A series of experimental results using the concept of covariance spectroscopy are presented.

  17. Imaging with INTEGRAL. [instrument for fine spectroscopy of celestial gamma-ray sources

    NASA Technical Reports Server (NTRS)

    Dean, A. J.

    1993-01-01

    The INTEGRAL mission was proposed in response to the ESA M2 call for proposals and is dedicated to the fine spectroscopy and imaging of celestial gamma-ray sources in the energy range 15 keV to 10 MeV. Cosmic gamma-rays are emitted on a wide range of angular scales and structures for a diverse population of astronomical objects. The emission, which includes discrete spectral lines and continuum radiation is derived from point sources, localized regions, as well as a diffuse band along the Galactic plane. Much of the gamma-ray sky is composed from transient phenomena which range from the few second timescale associated with gamma-ray bursts to larger lived events lasting some days or more. These class of events pose the challenge of firstly identification and secondly that of precise positional location of 'random' short lived events which arrive isotropically. In this article the imaging requirements are evaluated in light of current observational astronomical data and practical solutions for the INTEGRAL telescope are discussed. Some of the key problems are highlighted.

  18. Identification of lunar rock types and search for polar ice by gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Metzger, Albert E.; Drake, Darrell M.

    1990-01-01

    This paper examines the possibility of mapping the surface composition of the moon from an orbiting spin-stabilized spacecraft, using gamma ray spectroscopy and a cooled germanium solid-state device as a detector. A design for accommodating the germanium detector gamma ray spectrometer was devised, and the detection sensitivity was applied to typical lunar-rock compositions. For sets comprising nine highland and 16 mare types, the most useful elements were found to be Mg, Al, K, Ti, Fe, U, and Th. An analysis of the expected instrument response to the gamma ray and neutron fluxes of water ice indicated that a neutron mode added to the spectrometer will be more sensitive than the gamma ray mode to the possible presence of polar ice. It was calculated that, with a pair of selected neutron absorbers and a model which provides that 2.5 percent of the area above 75-deg latitude is occupied by trapping sites, the instrument will provide a 1-yr mission detection limit of 0.056 percent H2O by weight for each polar region.

  19. Line and continuum spectroscopy as diagnostic tools for gamma ray bursts

    SciTech Connect

    Liang, E.P.

    1990-12-01

    We review the theoretical framework of both line and continuum spectra formation in gamma ray bursts. These include the cyclotron features at 10's of keV, redshifted annihilation features at {approximately}400 keV, as well as other potentially detectable nuclear transition lines, atomic x-ray lines, proton cyclotron lines and plasma oscillation lines. By combining the parameters derived from line and continuum modeling we can try to reconstruct the location, geometry and physical conditions of the burst emission region, thereby constraining and discriminating the astrophysical models. Hence spectroscopy with current and future generations of detectors should provide powerful diagnostic tools for gamma ray bursters. 48 refs., 10 figs., 4 tabs.

  20. Perspectives for neutron and gamma spectroscopy in high power laser driven experiments at ELI-NP

    NASA Astrophysics Data System (ADS)

    Negoita, F.; Gugiu, M.; Petrascu, H.; Petrone, C.; Pietreanu, D.; Fuchs, J.; Chen, S.; Higginson, D.; Vassura, L.; Hannachi, F.; Tarisien, M.; Versteegen, M.; Antici, P.; Balabanski, D.; Balascuta, S.; Cernaianu, M.; Dancus, I.; Gales, S.; Neagu, L.; Petcu, C.; Risca, M.; Toma, M.; Turcu, E.; Ursescu, D.

    2015-02-01

    The measurement of energy spectra of neutrons and gamma rays emitted by nuclei, together with charge particles spectroscopy, are the main tools for understanding nuclear phenomena occurring also in high power laser driven experiments. However, the large number of particles emitted in a very short time, in particular the strong X-rays flash produced in laser-target interaction, impose adaptation of technique currently used in nuclear physics experiment at accelerator based facilities. These aspects are discussed (Section 1) in the context of proposed studies at high power laser system of ELI-NP. Preliminary results from two experiments performed at Titan (LLNL) and ELFIE (LULI) facilities using plastic scintillators for neutron detection (Section 2) and LaBr3(Ce) scintillators for gamma detection (Section 3) are presented demonstrating the capabilities and the limitations of the employed methods. Possible improvements of these spectroscopic methods and their proposed implementation at ELI-NP will be discussed as well in the last section.

  1. Time-resolved spectroscopy measurements of hydrogen-alpha, -beta, and -gamma emissions

    SciTech Connect

    Parigger, Christian G.; Dackman, Matthew; Hornkohl, James O

    2008-11-01

    Hydrogen emission spectroscopy results are reported following laser-induced optical breakdown with infrared Nd:YAG laser radiation focused into a pulsed methane flow. Measurements of Stark-broadened atomic hydrogen-alpha, -beta, and -gamma lines show electron number densities of 0.3 to 4x10{sup 17} cm{sup -3} for time delays of 2.1 to 0.4 {mu}s after laser-induced optical breakdown. In methane flow, recombination molecular spectra of the {delta}{nu}=+2 progression of the C2 Swan system are discernable in the H{beta} and H{gamma} plasma emissions within the first few microseconds. The recorded atomic spectra indicate the occurrence of hydrogen self-absorption for pulsed CH4 flow pressures of 2.7x10{sup 5} Pa (25 psig) and 6.5x10{sup 5} Pa (80 psig)

  2. Time-resolved spectroscopy measurements of hydrogen-alpha, -beta, and -gamma emissions.

    PubMed

    Parigger, Christian G; Dackman, Matthew; Hornkohl, James O

    2008-11-01

    Hydrogen emission spectroscopy results are reported following laser-induced optical breakdown with infrared Nd:YAG laser radiation focused into a pulsed methane flow. Measurements of Stark-broadened atomic hydrogen-alpha, -beta, and -gamma lines show electron number densities of 0.3 to 4x10(17) cm(-3) for time delays of 2.1 to 0.4 micros after laser-induced optical breakdown. In methane flow, recombination molecular spectra of the Delta nu = +2 progression of the C(2) Swan system are discernable in the H(beta) and H(gamma) plasma emissions within the first few microseconds. The recorded atomic spectra indicate the occurrence of hydrogen self-absorption for pulsed CH(4) flow pressures of 2.7x10(5) Pa (25 psig) and 6.5x10(5) Pa (80 psig). PMID:19122690

  3. BATSE gamma-ray burst line search. 1: Search for narrow lines in spectroscopy detector data

    NASA Technical Reports Server (NTRS)

    Palmer, David M.; Teegarden, Bonnard J.; Schaefer, Bradley E.; Cline, Thomas L.; Band, David L.; Ford, Lyle A.; Matteson, James L.; Paciesas, William S.; Pendleton, Geoffrey N.; Briggs, Michael S.

    1994-01-01

    Analysis of data from the Spectroscopy Detectors (SDs) of the Burst and Transient Source Experiment (BATSE) on the Compton Gamma Ray Observatory (GRO) has found no convincing line features in the spectra of gamma-ray bursts (GRBs) in almost 3 years of operation, in contrast to expectations based on results from other experiments. In this Letter we discuss the visual search for narrow lines in the SD data. The search has examined 192 bursts, of which approximately 18 were intense enough that lines similar to those seen by instruments on the Ginga satellite would have been visible between approximately 20 and approximately 100 keV. A simplified calculation shows that the BATSE and Ginga results are consistent at the 13% level.

  4. Comparison of in situ and laboratory gamma spectroscopy of natural radionuclides in desert soil.

    PubMed

    Benke, R R; Kearfott, K J

    1997-08-01

    In situ and laboratory gamma spectroscopy were used to characterize natural background levels of radiation in the soil at eight sites around the Yucca Mountain Range. The purpose of this practical field analysis was to determine if published empirical in situ calibration factors would yield accurate quantitative specific activities (Bq kg(-1)) in a desert environment. Corrections were made to the in situ calibration factors to account for the on-axis response of a detector with a thin beryllium end window. The in situ gamma spectroscopy results were compared to laboratory gamma spectroscopy of soil samples gathered from each site. Five natural radionuclides were considered: 40K, 214Pb, 214Bi, 208Tl, and 228Ac. The in situ determined specific activities were consistently within +/-15% of the laboratory soil sample results. A quantitative discussion of the factors contributing to the uncertainty in the in situ and laboratory results is included. Analysis on the specific activity data using statistical hypothesis tests determined that three nuclides, 214Pb, 214Bi, and 228Ac showed a weak site dependence while the other two nuclides, 40K and 208Tl, did not exhibit a site dependence. Differing radiation background levels from site to site along with in situ and laboratory uncertainties in excess of 10% are two factors that account for the weak site dependence. Despite the good correlation between data, it was recommended that the in situ detector be calibrated by a detector-specific Monte Carlo code which would accurately model more complex geometries and source distributions. PMID:9228170

  5. Study of asymmetries of Cd(Zn)Te devices investigated using photo-induced current transient spectroscopy, Rutherford backscattering, surface photo-voltage spectroscopy, and gamma ray spectroscopies

    SciTech Connect

    Crocco, J.; Bensalah, H.; Zheng, Q.; Dieguez, E.; Corregidor, V.; Avles, E.; Castaldini, A.; Fraboni, B.; Cavalcoli, D.; Cavallini, A.; Vela, O.

    2012-10-01

    Despite these recent advancements in preparing the surface of Cd(Zn)Te devices for detector applications, large asymmetries in the electronic properties of planar Cd(Zn)Te detectors are common. Furthermore, for the development of patterned electrode geometries, selection of each electrode surface is crucial for minimizing dark current in the device. This investigation presented here has been carried out with three objectives. Each objective is oriented towards establishing reliable methods for the selection of the anode and cathode surfaces independent of the crystallographic orientation. The objectives of this study are (i) investigate how the asymmetry in I-V characteristics of Cd(Zn)Te devices may be associated with the TeO2 interfacial layer using Rutherford backscattering to study the structure at the Au-Cd(Zn)Te interface, (ii) develop an understanding of how the concentration of the active traps in Cd(Zn)Te varies with the external bias, and (iii) propose non-destructive methods for selection of the anode and cathode which are independent of crystallographic orientation. The spectroscopic methods employed in this investigation include Rutherford backscattering spectroscopy, photo-induced current transient spectroscopy, and surface photo-voltage spectroscopy, as well as gamma ray spectroscopy to demonstrate the influence on detector properties.

  6. Concentration of liquid sample for gamma-ray spectroscopy with ultrasonic nebulization

    NASA Astrophysics Data System (ADS)

    Kim, Jungsoon; Kim, Jihyang; Jung, Jihee; Kim, Moojoon; Ha, Kanglyeol

    2015-07-01

    Radionuclide analysis of sea water is necessary to monitor environmental contamination due to the radioactive substances from nuclear facilities. However, it is difficult to analyze the nuclides promptly with the conventional method of coprecipitation during emergencies because the method requires long precipitation times. In this study, an effective concentration method with ultrasonic nebulization was suggested for sea water samples. When a sea water sample of 40 L was concentrated, 30 h was required with the conventional method, whereas it took less than 11 h with the suggested method. The validity of the suggested method was verified by gamma-ray spectroscopy.

  7. Gamma-ray-spectroscopy following high-flux 14-MeV neutron activation

    SciTech Connect

    Williams, R.E.

    1981-10-12

    The Rotating Target Neutron Source (RTNS-I), a high-intensity source of 14-MeV neutrons at the Lawrence Livermore National Laboratory (LLNL), has been used for applications in activation analysis, inertial-confinement-fusion diagnostic development, and fission decay-heat studies. The fast-neutron flux from the RTNS-I is at least 50 times the maximum fluxes available from typical neutron generators, making these applications possible. Facilities and procedures necessary for gamma-ray spectroscopy of samples irradiated at the RTNS-I were developed.

  8. Bismuth germanate's role in the new revolution in gamma-ray spectroscopy

    SciTech Connect

    Johnson, N.R.; Baktash, C.; Lee, I.Y.

    1983-01-01

    Some of the considerations on how to effectively incorporate bismuth germanate into complex detection systems are covered, and some of these new systems now in operation or under construction are discussed. Significant achievements in gamma ray spectroscopy are reviewed as well as some recent results based on data taken with coincidence arrays of germanium detectors and Compton-suppression spectrometers. Then the first impact of bismuth germanate detectors on our understanding of the properties of nuclei that have high energy and very high angular momentum states are addressed. (LEW)

  9. Solar abundances from gamma-ray spectroscopy - Comparisons with energetic particle, photospheric, and coronal abundances

    NASA Technical Reports Server (NTRS)

    Murphy, R. J.; Ramaty, R.; Reames, D. V.; Kozlovsky, B.

    1991-01-01

    Accelerated particle and ambient gas abundances have been derived using solar flare gamma-ray spectroscopy. The results with photospheric and coronal abundances, as well as with solar energetic particle abundances. This is the first time that the composition of accelerated particles interacting in an astrophysical source has been compared with the composition of particles escaping from the source. The analysis shows that the derived composition of the accelerated particles is different from the composition of particles observed in large proton flares; rather, it resembles the composition observed in He-3-rich flares. The analysis also suggests an ambient gas composition which differs from the composition of both the photosphere and the corona.

  10. Synthesis and Proton NMR Spectroscopy of Intra-Vesicular Gamma-Aminobutyric Acid (GABA)*

    PubMed Central

    Wang, Luke Y.-J.; Tong, Rong; Kohane, Daniel S.

    2014-01-01

    We report the synthesis of vesicles containing gamma-aminobutyric acid (GABA), and their proton nuclear magnetic resonance (1H NMR) spectra. These vesicles were constructed to more closely mimic the intracellular environment wherein GABA exists. For this study, these GABA-containing vesicles were examined under 1H NMR as a potential platform for future studies on the differences between aqueous phantoms, ex vivo brain extracts, and in vivo magnetic resonance spectroscopy results. We found that intra-vesicular GABA faithfully yielded the chemical shifts and J-coupling constants of free aqueous GABA, alongside the chemical shift signals of the vesicle wall. PMID:24109882

  11. Obelix, a new low-background HPGe at Modane Underground Laboratory

    SciTech Connect

    Loaiza, P.; Piquemal, F.; Warot, G.; Zampaolo, M.

    2015-08-17

    An ultra-low background coaxial HPGe detector for gamma-ray spectrometry with a relative efficiency of 160%, corresponding to a 600 cm{sup 3} Ge crystal, was installed at the Laboratoire Souterrain de Modane, France (4800 m.w.e). To reduce the instrinsic detector background, all parts involved in the detector cryostat were selected for their low radioactivity contamination. A shielding, composed of an inner layer of roman lead and an external layer of regular lead was installed, together with a system to reduce the Rn level inside the sample chamber. The shielding was designed to allow the measurement of Marinelli-shaped samples. We present the constructional details which lead to a remarkable low detector background of 73 cts/kg·d in [40, 3000] keV. Measured samples showed that sensitivities about 100 μBq/kg in {sup 226}Ra and {sup 228}Th are reached for samples of some kg and 30 days of lifetime.

  12. Digital Pulse-Shape Discrimination Applied to an Ultra-Low-Background Gas-Proportional Counting System: First Results

    SciTech Connect

    Aalseth, Craig E.; Day, Anthony R.; Fuller, Erin S.; Hoppe, Eric W.; Keillor, Martin E.; Mace, Emily K.; Myers, A. W.; Overman, Cory T.; Panisko, Mark E.; Seifert, Allen; Warren, Glen A.; Williams, Richard M.

    2013-05-01

    Abstract A new ultra-low-background proportional counter (ULBPC) design was recently developed at Pacific Northwest National Laboratory (PNNL). This design, along with an ultra-low-background counting system (ULBCS) which provides passive and active shielding with radon exclusion, has been developed to complement a new shallow underground laboratory (~30 meters water-equivalent) constructed at PNNL. After these steps to mitigate dominant backgrounds (cosmic rays, external gamma-rays, radioactivity in materials), remaining background events do not exclusively arise from ionization of the proportional counter gas. Digital pulse-shape discrimination (PSD) is thus employed to further improve measurement sensitivity. In this work, a template shape is generated for each individual sample measurement of interest, a "self-calibrating" template. Differences in event topology can also cause differences in pulse shape. In this work, the temporal region analyzed for each event is refined to maximize background discrimination while avoiding unwanted sensitivity to event topology. This digital PSD method is applied to sample and background data, and initial measurement results from a biofuel methane sample are presented in the context of low-background measurements currently being developed.

  13. Gamma ray spectroscopy at high energy and high time resolution at JET.

    PubMed

    Tardocchi, M; Proverbio, L I; Gorini, G; Grosso, G; Locatelli, M; Chugonov, I N; Gin, D B; Shevelev, A E; Murari, A; Kiptily, V G; Syme, B; Fernandes, A M; Pereira, R C; Sousa, J

    2008-10-01

    In fusion plasmas gamma ray emission is caused by reactions of fast particles, such as fusion alpha particles, with impurities. Gamma ray spectroscopy at JET has provided valuable diagnostic information on fast fuel as well as fusion product ions. Improvements of these measurements are needed to fully exploit the flux increase provided by future high power experiments at JET and ITER. Limiting aspects are, for instance, the count rate capability due to a high neutron/gamma background combined with slow detector response and a modest energy resolution due to the low light yield of the scintillators. This paper describes the solutions developed for achieving higher energy resolution, signal to background, and time resolution. The detector design is described based on the new BrLa3 scintillator crystal. The paper will focus on hardware development, including a photomultiplier tube capable of stable operation at counting rate as high as 1 MHz, the magnetic shielding, and the fast digital data acquisition system. PMID:19068513

  14. Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

    SciTech Connect

    Ludewigt, Bernhard; Mozin, Vladimir; Campbell, Luke; Favalli, Andrea; Alan W. Hunt; Reedy, Edward T.E.; Seipel, Heather

    2015-06-01

    High-­energy, beta-delayed gamma-­ray spectroscopy is a potential, non-­destructive assay techniques for the independent verification of declared quantities of special nuclear materials at key stages of the fuel cycle and for directly assaying nuclear material inventories for spent fuel handling, interim storage, reprocessing facilities, repository sites, and final disposal. Other potential applications include determination of MOX fuel composition, characterization of nuclear waste packages, and challenges in homeland security and arms control verification. Experimental measurements were performed to evaluate fission fragment yields, to test methods for determining isotopic fractions, and to benchmark the modeling code package. Experimental measurement campaigns were carried out at the IAC using a photo-­neutron source and at OSU using a thermal neutron beam from the TRIGA reactor to characterize the emission of high-­energy delayed gamma rays from 235U, 239Pu, and 241Pu targets following neutron induced fission. Data were collected for pure and combined targets for several irradiation/spectroscopy cycle times ranging from 10/10 seconds to 15/30 minutes.The delayed gamma-ray signature of 241Pu, a significant fissile constituent in spent fuel, was measured and compared to 239Pu. The 241Pu/239Pu ratios varied between 0.5 and 1.2 for ten prominent lines in the 2700-­3600 keV energy range. Such significant differences in relative peak intensities make it possible to determine relative fractions of these isotopes in a mixed sample. A method for determining fission product yields by fitting the energy and time dependence of the delayed gamma-­ray emission was developed and demonstrated on a limited 235U data set. De-­convolution methods for determining fissile fractions were developed and tested on the experimental data. The use of high count-­rate LaBr3 detectors

  15. Experimental investigation of silicon photomultipliers as compact light readout systems for gamma-ray spectroscopy applications in fusion plasmas.

    PubMed

    Nocente, M; Fazzi, A; Tardocchi, M; Cazzaniga, C; Lorenzoli, M; Pirovano, C; Rebai, M; Uboldi, C; Varoli, V; Gorini, G

    2014-11-01

    A matrix of Silicon Photo Multipliers has been developed for light readout from a large area 1 in. × 1 in. LaBr3 crystal. The system has been characterized in the laboratory and its performance compared to that of a conventional photo multiplier tube. A pulse duration of 100 ns was achieved, which opens up to spectroscopy applications at high counting rates. The energy resolution measured using radioactive sources extrapolates to 3%-4% in the energy range Eγ = 3-5 MeV, enabling gamma-ray spectroscopy measurements at good energy resolution. The results reported here are of relevance in view of the development of compact gamma-ray detectors with spectroscopy capabilities, such as an enhanced gamma-ray camera for high power fusion plasmas, where the use of photomultiplier is impeded by space limitation and sensitivity to magnetic fields. PMID:25430287

  16. Experimental investigation of silicon photomultipliers as compact light readout systems for gamma-ray spectroscopy applications in fusion plasmas

    SciTech Connect

    Nocente, M. Gorini, G.; Fazzi, A.; Lorenzoli, M.; Pirovano, C.; Tardocchi, M.; Cazzaniga, C.; Rebai, M.; Uboldi, C.; Varoli, V.

    2014-11-15

    A matrix of Silicon Photo Multipliers has been developed for light readout from a large area 1 in. × 1 in. LaBr{sub 3} crystal. The system has been characterized in the laboratory and its performance compared to that of a conventional photo multiplier tube. A pulse duration of 100 ns was achieved, which opens up to spectroscopy applications at high counting rates. The energy resolution measured using radioactive sources extrapolates to 3%–4% in the energy range E{sub γ} = 3–5 MeV, enabling gamma-ray spectroscopy measurements at good energy resolution. The results reported here are of relevance in view of the development of compact gamma-ray detectors with spectroscopy capabilities, such as an enhanced gamma-ray camera for high power fusion plasmas, where the use of photomultiplier is impeded by space limitation and sensitivity to magnetic fields.

  17. Simulation of background reduction and Compton suppression in a low-background HPGe spectrometer at a surface laboratory

    NASA Astrophysics Data System (ADS)

    Niu, Shun-Li; Cai, Xiao; Wu, Zhen-Zhong; Liu, Yi; Xie, Yu-Guang; Yu, Bo-Xiang; Wang, Zhi-Gang; Fang, Jian; Sun, Xi-Lei; Sun, Li-Jun; Liu, Ying-Biao; Gao, Long; Zhang, Xuan; Zhao, Hang; Zhou, Li; Lü, Jun-Guang; Hu, Tao

    2015-08-01

    High-purity germanium (HPGe) detectors are well suited to analyse the radioactivity of samples. In order to reduce the environmental background for an ultra-low background HPGe spectrometer, low-activity lead and oxygen free copper are installed outside the probe to shield from gamma radiation, with an outer plastic scintillator to veto cosmic rays, and an anti-Compton detector to improve the peak-to-Compton ratio. Using Geant4 tools and taking into account a detailed description of the detector, we optimize the sizes of these detectors to reach the design requirements. A set of experimental data from an existing HPGe spectrometer was used to compare with the simulation. For the future low-background HPGe detector simulation, considering different thicknesses of BGO crystals and anti-coincidence efficiency, the simulation results show that the optimal BGO thickness is 5.5 cm, and the peak-to-Compton ratio of 40K is raised to 1000 when the anti-coincidence efficiency is 0.85. In the background simulation, 15 cm oxygen-free copper plus 10 cm lead can reduce the environmental gamma rays to 0.0024 cps/100 cm3 Ge (50 keV-2.8 MeV), which is about 10-5 of the environmental background.

  18. Development of a low background test facility for the SPICA-SAFARI on-ground calibration

    NASA Astrophysics Data System (ADS)

    Dieleman, P.; Laauwen, W. M.; Ferrari, L.; Ferlet, M.; Vandenbussche, B.; Meinsma, L.; Huisman, R.

    2012-09-01

    SAFARI is a far-infrared camera to be launched in 2021 onboard the SPICA satellite. SAFARI offers imaging spectroscopy and imaging photometry in the wavelength range of 34 to 210 μm with detector NEP of 2•10-19 W/√Hz. A cryogenic test facility for SAFARI on-ground calibration and characterization is being developed. The main design driver is the required low background of a few attoWatts per pixel. This prohibits optical access to room temperature and hence all test equipment needs to be inside the cryostat at 4.5K. The instrument parameters to be verified are interfaces with the SPICA satellite, sensitivity, alignment, image quality, spectral response, frequency calibration, and point spread function. The instrument sensitivity is calibrated by a calibration source providing a spatially homogeneous signal at the attoWatt level. This low light intensity is achieved by geometrical dilution of a 150K source to an integrating sphere. The beam quality and point spread function is measured by a pinhole/mask plate wheel, back-illuminated by a second integrating sphere. This sphere is fed by a stable wide-band source, providing spectral lines via a cryogenic etalon.

  19. High-performance gamma spectroscopy for equipment retrieval from Hanford high-level nuclear waste tanks

    NASA Astrophysics Data System (ADS)

    Troyer, Gary L.; Hillesand, K. E.; Goodwin, S. G.; Kessler, S. F.; Killian, E. W.; Legare, D.; Nelson, Joseph V., Jr.; Richard, R. F.; Nordquist, E. M.

    1999-01-01

    The cleanup of high level defense nuclear waste at the Hanford site presents several progressive challenges. Among these is the removal and disposal of various components from buried active waste tanks to allow new equipment insertion or hazards mitigation. A unique automated retrieval system at the tank provides for retrieval, high pressure washing, inventory measurement, and containment for disposal. Key to the inventory measurement is a three detector HPGe high performance gamma spectroscopy system capable of recovering data at up to ninety per cent saturation (200,000 counts per second). Data recovery is based on a unique embedded electronic pulser and specialized software to report the inventory. Each of the detectors have different shielding specified through Monte Carlo simulation with the MCNP program. This shielding provides performance over a dynamic range of eight orders of magnitude. System description, calibration issues and operational experiences are discussed.

  20. In-Beam Gamma-ray Spectroscopy in the sdpf {sup 37}Ar Nucleus

    SciTech Connect

    Silveira, M. A. G.; Medina, N. H.; Seale, W. A.; Ribas, R. V.; Oliveira, J. R. B. de; Zilio, S.; Lenzi, S. M.; Napoli, D. R.; Marginean, N.; Vedova, F. Della; Farnea, E.; Ionescu-Bujor, M.; Iordachescu, A.

    2007-10-26

    The nucleus {sup 37}Ar has been studied with {gamma}-ray spectroscopy in the {sup 24}Mg({sup 16}O,2pn) reaction at a beam energy of 70 MeV. Twenty two new excited states up to an excitation energy of 13 MeV have been observed. We compare the first negative and positive parity yrast states with large-scale-shell-model calculations using the Antoine code and the SDPF interaction, considering the excitation of the 1d{sub 5/2},2s{sub 1/2} and 1d{sub 3/2} nucleons to 1f{sub 7/2} and 2p{sub 3/2} in the sdpf valence space.

  1. Cryogenic detector development at LLNL: ultraviolet x-ray, gamma-ray and biomolecule spectroscopy

    SciTech Connect

    Labov, S.E.; Frank, M.; le Grand, J.B.

    1997-08-12

    We are developing low-temperature detectors for optical, ultraviolet, X-ray, and gamma-ray spectroscopy, and for biomolecular mass spectrometry. We present development work on these detectors and materials analysis and biomolecular mass spectrometry. We have measured thin-film Nb/Al/Al2O3/AlNb superconducting tunnel junction (STJ) X-ray detectors in the 0.2 to 1 keV band with a range of different junction sizes and aluminum film thicknesses. In one case, we have achieved the statistical limit to the energy resolution of 13 eV FWHM at 227 eV with an output count rate of 20,600 cts/s.

  2. Low-Energy Study of Gamma-Ray Bursts Using Two BATSE Spectroscopy Detectors

    NASA Technical Reports Server (NTRS)

    Pangia, Michael J.

    2002-01-01

    Gamma-ray bursts (GRBs) are energetic, short-duration emissions of gamma-rays from astronomical sources typically well beyond our galaxy. The Burst and Transient Source Experiment (BATSE) that was onboard NASA's Compton Gamma-Ray Observatory (CGRO) had detected an unprecedented 2704 GRBs during CGRO's nine-year mission. BATSE consisted of eight detector assemblies located at the corners of CGRO to give full sky coverage. Each assembly consisted of two detectors, a Large Area Detector (LAD) and a Spectroscopy Detector (SD). In determining the detail features of GRBs, the degree to which they possess a low-energy component (approx. 10 keV) is of interest. Preece has developed a method to study the low-energy characteristics and concluded that 14% of the 86 bright GRBs they studied had a definite low-energy component, referred to as a low-energy excess. Their study, and the present study as well, needed to use SD data, because it extends down to the low-energy range when operating in a high-gain mode. For their study, low-energy data was used from just one SD. To better quantify the low-energy behavior, this study will consider bursts for which two SDs satisfy the same criteria as used by Preece. The procedure developed by Preece to study the low-energy aspects of GRBs with BATSE data is to fit the data to a representative spectral function. In particular, two components are used, one corresponding to the low-energy component, and another representing the main part of the spectrum. The low-energy function used is the optically thin thermal bremsstrahlung (OTTB) model.

  3. Perspectives for neutron and gamma spectroscopy in high power laser driven experiments at ELI-NP

    SciTech Connect

    Negoita, F. Gugiu, M. Petrascu, H. Petrone, C. Pietreanu, D.; Fuchs, J.; Chen, S.; Higginson, D.; Vassura, L.; Hannachi, F.; Tarisien, M.; Versteegen, M.; Antici, P.; Balabanski, D.; Balascuta, S.; Cernaianu, M.; Dancus, I.; Gales, S.; Neagu, L.; Petcu, C.; and others

    2015-02-24

    The measurement of energy spectra of neutrons and gamma rays emitted by nuclei, together with charge particles spectroscopy, are the main tools for understanding nuclear phenomena occurring also in high power laser driven experiments. However, the large number of particles emitted in a very short time, in particular the strong X-rays flash produced in laser-target interaction, impose adaptation of technique currently used in nuclear physics experiment at accelerator based facilities. These aspects are discussed (Section 1) in the context of proposed studies at high power laser system of ELI-NP. Preliminary results from two experiments performed at Titan (LLNL) and ELFIE (LULI) facilities using plastic scintillators for neutron detection (Section 2) and LaBr{sub 3}(Ce) scintillators for gamma detection (Section 3) are presented demonstrating the capabilities and the limitations of the employed methods. Possible improvements of these spectroscopic methods and their proposed implementation at ELI-NP will be discussed as well in the last section.

  4. High-precision gamma-ray spectroscopy for enhancing production and application of medical isotopes

    NASA Astrophysics Data System (ADS)

    McCutchan, E. A.; Sonzogni, A. A.; Smith, S. V.; Muench, L.; Nino, M.; Greene, J. P.; Carpenter, M. P.; Zhu, S.; Chillery, T.; Chowdhury, P.; Harding, R.; Lister, C. J.

    2015-10-01

    Nuclear medicine is a field which requires precise decay data for use in planning radionuclide production and in imaging and therapeutic applications. To address deficiencies in decay data, sources of medical isotopes were produced and purified at the Brookhaven Linear Isotope Producer (BLIP) then shipped to Argonne National Laboratory where high-precision, gamma-ray measurements were performed using Gammasphere. New decay schemes for a number of PET isotopes and the impact on dose calculations will be presented. To investigate the production of next-generation theranostic or radiotherapeutic isotopes, cross section measurements with high energy protons have also been explored at BLIP. The 100-200 MeV proton energy regime is relatively unexplored for isotope production, thus offering high discovery potential but at the same time a challenging analysis due to the large number of open channels at these energies. Results of cross sections deduced from Compton-suppressed, coincidence gamma-ray spectroscopy performed at Lowell will be presented, focusing on the production of platinum isotopes by irradiating natural platinum foils with 100 to 200 MeV protons. DOE Isotope Program is acknowledged for funding ST5001030. Work supported by the US DOE under Grant DE-FG02-94ER40848 and Contracts DE-AC02-98CH10946 and DE-AC02-06CH11357.

  5. Investigation of LaBr3:Ce probe for gamma-ray spectroscopy and dosimetry

    NASA Astrophysics Data System (ADS)

    Maghraby, Ahmed M.; Alzimami, K. S.; Alkhorayef, M. A.; Alsafi, K. G.; Ma, A.; Alfuraih, A. A.; Alghamdi, A. A.; Spyrou, N. M.

    2014-02-01

    The main thrust of this work is the investigation of performance of relatively new commercial LaBr3:Ce probe (Inspector 1000™ with LaBr3:Ce crystal) for gamma-ray spectroscopy and dosimetry measurements in comparison to LaCl3:Ce and NaI:Tl scintillators. The crystals were irradiated by a wide range of energies (57Co, 22Na, 18F, 137Cs and 60Co). The study involved recording of detected spectra and measurement of energy resolution, photopeak efficiency, internal radioactivity measurements as well as dose rate. The Monte Carlo package, Geant4 Application for Tomographic Emission (GATE) was used to validate the experiments. Overall results showed very good agreement between the measurements and the simulations. The LaBr3:Ce crystal has excellent energy resolution, energy resolutions of (3.37±0.05)% and (2.98±0.07)% for a 137Cs 662 keV and a 60Co 1332 keV gamma-ray point sources respectively, were recorded. The disadvantage of the lanthanum halide scintillators is their internal radioactivity. Inspector 1000™ with LaBr3:Ce scintillator has shown an accurate and quick dose measurements at Positron Emission Tomography (PET) Units which allows accurate assessment of the radiation dose received by staff members compared to the use of electronic personal dosimeters (EPD).

  6. Distance dependent quenching and gamma-ray spectroscopy in tin-loaded polystyrene scintillators

    DOE PAGESBeta

    Feng, Patrick L; Mengesha, Wondwosen; Anstey, Mitchell R.; Cordaro, Joseph Gabriel

    2016-02-01

    In this study, we report the synthesis and inclusion of rationally designed organotin compounds in polystyrene matrices as a route towards plastic scintillators capable of gamma-ray spectroscopy. Tin loading ratios of up to 15% w/w have been incorporated, resulting in photopeak energy resolution values as low as 10.9% for 662 keV gamma-rays. Scintillator constituents were selected based upon a previously reported distance-dependent quenching mechanism. Data obtained using UV-Vis and photoluminescence measurements are consistent with this phenomenon and are correlated with the steric and electronic properties of the respective organotin complexes. We also report fast scintillation decay behavior that is comparablemore » to the quenched scintillators 0.5% trans-stilbene doped bibenzyl and the commercial plastic scintillator BC-422Q-1%. These observations are discussed in the context of practical considerations such as optical transparency, ease-of-preparation/scale-up, and total scintillator cost.« less

  7. Raman spectroscopy of 2-hydroxyethyl methacrylate-acrylamide copolymer using gamma irradiation for crosslinking

    SciTech Connect

    Goheen, Steven C.; Saunders, Rachel M.; Davis, Rachel M.; Harvey, Scott D.; Olsen, Peter C.

    2006-02-18

    A copolymer hydrogel was made by mixing acrylamide and 2-hydroxyethyl methacrylate monomers in water and polymerizing with gamma irradiation. The progress of polymerization and the vibrational structure of the hydrogel was examined using Raman spectroscopy. Raman spectra indicated that the co-polymer has a molecular structure different from polyacrylamide or the individual monomers. The Raman data also indicate the presence of crosslinking at the C=O, NH2 and OH side chains. The spectra further suggest the continuous lengthening of the backbone of the polymers with increasing gamma dose. This is shown as the increase in C-C modes as C=C vibrations decrease. Raman spectra changed most dramatically as the monomer mixture became a gel at a dose of approximately 320 Gy. Spectral differences were subtler with doses exceeding 640 Gy, although chain lengthening continued beyond 1500 Gy. Potential applications of the copolymer hydrogel include reconstructive tissue as well as a standard material for radiation protection dosimetry. Results are discussed in relation to other potential applications of this polymer and dose-dependent changes in the Raman spectrum.

  8. Phantom experiment and calculation for in vivo 10boron analysis by prompt gamma ray spectroscopy.

    PubMed

    Matsumoto, T; Aoki, M; Aizawa, O

    1991-03-01

    In order to determine 10B concentrations in a tumour in vivo without injuring tissues, phantom experiments and calculations were carried out for boron neutron capture therapy. The experiment was based on prompt gamma ray spectroscopy and a single-crystal silicon-filtered neutron beam from a TRIGA-II reactor. Calibration curves to determine the 10B concentrations in the tumours were experimentally generated from known 10B values for simulated tumours with various volumes in a phantom. The 10B distributions in a tumour were also investigated and it was possible to distinguish the tumour with 10B from normal tissue without 10B. In addition, the 10B concentrations were estimated by calculations. A two-dimensional discrete ordinate transport code, DOT3.5, was employed for the calculations of the neutron fluence rate distributions in a phantom. The number of incidental gamma rays entering a germanium detector, which were produced in a tumour as a result of neutron reaction, were calculated by an analytical method. The results were in good agreement with the experiments. PMID:2038605

  9. A weak magnetism observed in SnO2 doped with Fe by means of Perturbed Gamma-Gamma Angular Correlation and Mössbauer Spectroscopy

    NASA Astrophysics Data System (ADS)

    Ramos, J. M.; Carbonari, A. W.; Martucci, T.; Costa, M. S.; Cabrera-Pasca, G. A.; Macedo, M. A. V.; Saxena, R. N.

    Nano-structured samples of SnO2 doped with Fe prepared by the sol-gel method were studied by the Perturbed Gamma-Gamma Angular Correlation (PAC) Spectroscopy using 111In (111Cd) probe nuclei as well as by 57Fe Mšssbauer spectroscopy. The samples were prepared from very pure metallic Sn and Fe. Carrier-free 111In nuclei were introduced during the sol-gel process of sample preparation for PAC measurements. The PAC measurements were carried out after annealing the samples at different temperatures and the results show a combined electric quadrupole and magnetic dipole interaction for probe nuclei that do not occupy the regular Sn sites. The hyperfine parameters revealed weak magnetic interactions.

  10. Gamma-induced positron annihilation spectroscopy and application to radiation-damaged alloys

    NASA Astrophysics Data System (ADS)

    Wells, D. P.; Hunt, A. W.; Tchelidze, L.; Kumar, J.; Smith, K.; Thompson, S.; Selim, F.; Williams, J.; Harmon, J. F.; Maloy, S.; Roy, A.

    2006-06-01

    Radiation damage and other defect studies of materials are limited to thin samples because of inherent limitations of well-established techniques such as diffraction methods and traditional positron annihilation spectroscopy (PAS) [P. Hautojarvi, et al., Positrons in Solids, Springer, Berlin, 1979, K.G. Lynn, et al., Appl. Phys. Lett. 47 (1985) 239]. This limitation has greatly hampered industrial and in-situ applications. ISU has developed new methods that use pair-production to produce positrons throughout the volume of thick samples [F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 192 (2002) 197, F.A. Selim, D.P. Wells, et al., Nucl. Instru. Meth. A 495 (2002) 154, F.A. Selim, et al., J. Rad. Phys. Chem. 68 (2004) 427, F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 241 (2005) 253, A.W. Hunt, D.P. Wells, et al., Nucl. Instr. and Meth. B. 241 (2005) 262]. Unlike prior work at other laboratories that use bremsstrahlung beams to create positron beams (via pair-production) that are then directed at a sample of interest, we produce electron-positron pairs directly in samples of interest, and eliminate the intermediate step of a positron beam and its attendant penetrability limitations. Our methods include accelerator-based bremsstrahlung-induced pair-production in the sample for positron annihilation energy spectroscopy measurements (PAES), coincident proton-capture gamma-rays (where one of the gammas is used for pair-production in the sample) for positron annihilation lifetime spectroscopy (PALS), or photo-nuclear activation of samples for either type of measurement. The positrons subsequently annihilate with sample electrons, emitting coincident 511 keV gamma-rays [F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 192 (2002) 197, F.A. Selim, D.P. Wells, et al., Nucl. Instru. Meth. A 495 (2002) 154, F.A. Selim, et al., J. Rad. Phys. Chem. 68 (2004) 427, F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 241 (2005) 253, A.W. Hunt, D

  11. Photon-induced positron annihilation lifetime spectroscopy using ultrashort laser-Compton-scattered gamma-ray pulses

    SciTech Connect

    Taira, Y.; Toyokawa, H.; Kuroda, R.; Yamamoto, N.; Adachi, M.; Tanaka, S.; Katoh, M.

    2013-05-15

    High-energy ultrashort gamma-ray pulses can be generated via laser Compton scattering with 90 Degree-Sign collisions at the UVSOR-II electron storage ring. As an applied study of ultrashort gamma-ray pulses, a new photon-induced positron annihilation lifetime spectroscopy approach has been developed. Ultrashort gamma-ray pulses with a maximum energy of 6.6 MeV and pulse width of 2.2 ps created positrons throughout bulk lead via pair production. Annihilation gamma rays were detected by a BaF{sub 2} scintillator mounted on a photomultiplier tube. A positron lifetime spectrum was obtained by measuring the time difference between the RF frequency of the electron storage ring and the detection time of the annihilation gamma rays. We calculated the response of the BaF{sub 2} scintillator and the time jitter caused by the variation in the total path length of the ultrashort gamma-ray pulses, annihilation gamma rays, and scintillation light using a Monte Carlo simulation code. The positron lifetime for bulk lead was successfully measured.

  12. Photon-induced positron annihilation lifetime spectroscopy using ultrashort laser-Compton-scattered gamma-ray pulses.

    PubMed

    Taira, Y; Toyokawa, H; Kuroda, R; Yamamoto, N; Adachi, M; Tanaka, S; Katoh, M

    2013-05-01

    High-energy ultrashort gamma-ray pulses can be generated via laser Compton scattering with 90° collisions at the UVSOR-II electron storage ring. As an applied study of ultrashort gamma-ray pulses, a new photon-induced positron annihilation lifetime spectroscopy approach has been developed. Ultrashort gamma-ray pulses with a maximum energy of 6.6 MeV and pulse width of 2.2 ps created positrons throughout bulk lead via pair production. Annihilation gamma rays were detected by a BaF2 scintillator mounted on a photomultiplier tube. A positron lifetime spectrum was obtained by measuring the time difference between the RF frequency of the electron storage ring and the detection time of the annihilation gamma rays. We calculated the response of the BaF2 scintillator and the time jitter caused by the variation in the total path length of the ultrashort gamma-ray pulses, annihilation gamma rays, and scintillation light using a Monte Carlo simulation code. The positron lifetime for bulk lead was successfully measured. PMID:23742543

  13. Photon-induced positron annihilation lifetime spectroscopy using ultrashort laser-Compton-scattered gamma-ray pulses

    NASA Astrophysics Data System (ADS)

    Taira, Y.; Toyokawa, H.; Kuroda, R.; Yamamoto, N.; Adachi, M.; Tanaka, S.; Katoh, M.

    2013-05-01

    High-energy ultrashort gamma-ray pulses can be generated via laser Compton scattering with 90° collisions at the UVSOR-II electron storage ring. As an applied study of ultrashort gamma-ray pulses, a new photon-induced positron annihilation lifetime spectroscopy approach has been developed. Ultrashort gamma-ray pulses with a maximum energy of 6.6 MeV and pulse width of 2.2 ps created positrons throughout bulk lead via pair production. Annihilation gamma rays were detected by a BaF2 scintillator mounted on a photomultiplier tube. A positron lifetime spectrum was obtained by measuring the time difference between the RF frequency of the electron storage ring and the detection time of the annihilation gamma rays. We calculated the response of the BaF2 scintillator and the time jitter caused by the variation in the total path length of the ultrashort gamma-ray pulses, annihilation gamma rays, and scintillation light using a Monte Carlo simulation code. The positron lifetime for bulk lead was successfully measured.

  14. Comparative Gamma Spectroscopy with SrI2(Eu), GYGAG(Ce) and Bi-loaded Plastic Scintillators

    SciTech Connect

    Cherepy, N J

    2010-11-19

    We are developing new scintillator materials that offer potential for high resolution gamma ray spectroscopy at low cost. Single crystal SrI{sub 2}(Eu) offers {approx}3% resolution at 662 keV, in sizes of {approx}1 in{sup 3}. We have developed ceramics processing technology allowing us to achieve cubic inch scale transparent ceramic scintillators offering gamma spectroscopy performance superior to NaI(Tl). We fabricated a bismuth-loaded plastic scintillator that demonstrates energy resolution of {approx}8% at 662 keV in small sizes. Gamma ray spectroscopy can be used to identify the presence of weak radioactive sources within natural background. The ability to discriminate close-lying spectral lines is strongly dependent upon the energy resolution of the detector. In addition to excellent energy resolution, large volume detectors are needed to acquire sufficient events, for example, to identify a radioactive anomaly moving past a detector. We have employed a 'directed search' methodology for identifying potential scintillator materials candidates, resulting in the discovery of Europium-doped Strontium Iodide, SrI{sub 2}(Eu), Cerium-doped Gadolinium Garnet, GYGAG(Ce), and Bismuth-loaded Polymers. These scintillators possess very low self-radioactivity, offer energy resolution of 3-8% at 662 keV, and have potential to be grown cost-effectively to sizes similar to the most widely deployed gamma spectroscopy scintillator, Thallium-doped Sodium Iodide, NaI(Tl). In this study, gamma ray spectra of a variety of sources, were obtained employing SrI{sub 2}(Eu), GYGAG(Ce), Bi-loaded polymers, LaBr{sub 3}(Ce), and NaI(Tl). The effects of detector size, energy resolution, and background radioactivity (including self-radioactivity) on the ability to distinguish weak sources is quantified, based on a simple model, and qualitatively compared to laboratory data.

  15. Determination of environmental radiation flux and organ doses using in-situ gamma spectroscopy

    NASA Astrophysics Data System (ADS)

    Al-Ghamdi, Abdulrahman S.

    Contamination of buildings represent a unique problem during Decontamination and Decommissioning (D&D) of nuclear facilities. It is necessary to determine the long-lived radionuclides and their respective specific activities in building materials before the right D&D decision can be made. At the same time, radiation risk of workers or potential occupants in the facility must be assessed as part of the D&D process. The goal of this project was to develop a methodology of obtaining gamma radiation flux and organ doses from in-situ gamma spectroscopy. Algorithms were developed to simulate the response functions of the HPGe detector and to convert the spectra into photon fluences. A Monte Carlo code, MCNP4C, was used to simulate HPGe detector response and to develop the conversion algorithm. The simulated spectra obtained for an HPGe detector were converted to flux using the algorithm for various different geometries. The response functions of the detector are presented in this document for the gamma energies from 60 keV to 2.2 MeV. Published fluence-to-dose conversion coefficients were used to calculate organ doses and effective dose equivalent. We then tested the theory at a 100-MeV linear electron accelerator at Rensselaer Polytechnic Institute (RPI). Samples of the activated concrete walls and floor in the target room of the Linac facility as well as some steel samples were taken to quantify the specific activities of the structures. The results show that the most important long-lived radionuclides include 22 Na, 46Sc, 54 Mn, 57Co, 60 Co, 65Zn, 152 Eu and 154Eu, depending on the location and composition of the material. The specific activities at the Linac facility range from 1.15E-01 to 765.31 muCi/Kg. The annual effective dose equivalent was assessed to be 2.44 mSv y-1 (0.244 rem y-1 ), which is about 5% of the Annual EDE limits to workers.

  16. Gamma-ray burst and spectroscopy instrumentation development at the Goddard Space Flight Center

    NASA Technical Reports Server (NTRS)

    Teegarden, B. J.

    1986-01-01

    This paper summarizes the activities that are specifically related to the development of instrumentation for gamma-ray astronomy. Three programs are described: (1) the Gamma-Ray Imaging Spectrometer (GRIS), a balloon-borne array of seven germanium detectors for high-resolution spectrographic studies of persistent gamma-ray sources; (2) the Transient Gamma-Ray Spectrometer (TGRS), a single radiatively-cooled germanium detector for the spectrographic study of gamma-ray bursts, and (3) the Rapidly Moving Telescope (RMT), a ground-based optical telescope for the detection and study of short-lived optical transients, particularly those that occur in coincidence with gamma-ray bursts.

  17. Stimulus generation technique for code simulation of FPGA based gamma spectroscopy system

    NASA Astrophysics Data System (ADS)

    Rahman, Nur Aira Abd; Ramli, Abdul Rahman; Lombigit, Lojius; Abdullah, Nor Arymaswati; Khalid, Mohd Ashhar Hj

    2014-02-01

    The aim of this study is to develop a software that can systematically generate stimulus required for code simulation (functional and timing) of new digital processors in gamma spectroscopy system. Software must be able to produce stimulus that emulate ADC data of charge sensitive amplifier (CSA) output signal. Signal parameters such as pulse shape, amplitude, pulse width and count rate should be adjustable while allowing options such as pulse pile-up and random pulse events. To fulfill this objective, a pulse generator software PulseGEN has been developed. The software GUI is designed to operate in two modes, Single/Pile-Up Mode and Continuous Random Mode. Its ADC module simulates real-time ADC sampling. The output can be saved as input stimulus to test various functions of digital processors such as pulse height measurements, pile-up detection and correction, as well as random pulse detection and measurement that is similar to the actual real-time measurement. PulseGEN results have been compared and verified against commercial charge sensitive amplifier with NaI detector and NIM pulser.

  18. GRBSpec: a multi-observatory database for gamma-ray burst spectroscopy

    NASA Astrophysics Data System (ADS)

    de Ugarte Postigo, Antonio; Blazek, Martin; Janout, Petr; Sprimont, Pierre; Thöne, Christina C.; Gorosabel, Javier; Sánchez-Ramírez, Rubén.

    2014-07-01

    Gamma-ray bursts (GRBs) are the most luminous explosions in the Universe. They are produced during the collapse of massive stellar-sized objects, which create a black hole and eject material at ultra-relativistic speeds. They are unique tools to study the evolution of our Universe, as they are the only objects that, thanks to their extraordinary luminosity, can be observed during the complete history of star formation, from the era of reionisation to our days. One of the main tools to obtain information from GRBs and their environment is optical and near-infrared spectroscopy. After 17 years of studies spectroscopic data for around 300 events that have been collected. However, spectra were obtained by many groups, at different observatories, and using instruments of very different types, making data difficult to access, process and compare. Here we present GRBspec: A collaborative database that includes processed GRB spectra from multiple observatories and makes them available to the community. The website provides access to the datasets, allowing queries based not only on the observation characteristics but also on the properties of the GRB that was observed. Furthermore, the website provides visualisation and analysis tools, that allow the user to asses the quality of the data before downloading and even make data analysis online.

  19. A Multi-Contact, Low Capacitance HPGe Detector for High Rate Gamma Spectroscopy

    SciTech Connect

    Cox, Christopher

    2014-12-04

    The detection, identification and non-destructive assay of special nuclear materials and nuclear fission by-products are critically important activities in support of nuclear non-proliferation programs. Both national and international nuclear safeguard agencies recognize that current accounting methods for spent nuclear fuel are inadequate from a safeguards perspective. Radiation detection and analysis by gamma-ray spectroscopy is a key tool in this field, but no instrument exists that can deliver the required performance (energy resolution and detection sensitivity) in the presence of very high background count rates encountered in the nuclear safeguards arena. The work of this project addresses this critical need by developing a unique gamma-ray detector based on high purity germanium that has the previously unachievable property of operating in the 1 million counts-per-second range while achieving state-of-the-art energy resolution necessary to identify and analyze the isotopes of interest. The technical approach was to design and fabricate a germanium detector with multiple segmented electrodes coupled to multi-channel high rate spectroscopy electronics. Dividing the germanium detector’s signal electrode into smaller sections offers two advantages; firstly, the energy resolution of the detector is potentially improved, and secondly, the detector is able to operate at higher count rates. The design challenges included the following; determining the optimum electrode configuration to meet the stringent energy resolution and count rate requirements; determining the electronic noise (and therefore energy resolution) of the completed system after multiple signals are recombined; designing the germanium crystal housing and vacuum cryostat; and customizing electronics to perform the signal recombination function in real time. In this phase I work, commercial off-the-shelf electrostatic modeling software was used to develop the segmented germanium crystal geometry

  20. New Measurement of ^39Ar in Underground Argon with a Low Background Liquid Argon Detector

    NASA Astrophysics Data System (ADS)

    Xu, Jingke

    2012-03-01

    A low background liquid argon detector has been developed for sensitive measurements of the beta radioactive ^39Ar in argon from underground sources. The measurement is motivated by the need to improve on earlier studies that showed no sign of ^39Ar in certain sources of underground argon, but with a limited sensitivity of ˜ 5% relative to ^39Ar in atmospheric argon[1]. We will report preliminary measurements taken with the low background detector that was commissioned and operated at the Kimballton Underground Research Facility (KURF) in Virginia. A combination of passive and active background reduction techniques resulted in a very low background and a null result with sensitivity to ^39Ar less than 1% of atmospheric. The results confirm that underground argon is well suited for direct detection of dark matter WIMPs. [4pt] [1] D. Acosta-Kane et al., Nucl. Instr. Meth. A 587:46 (2008)

  1. Construction of a Shallow Underground Low-background Detector for a CTBT Radionuclide Laboratory

    SciTech Connect

    Forrester, Joel B.; Greenwood, Lawrence R.; Miley, Harry S.; Myers, Allan W.; Overman, Cory T.

    2013-05-01

    The International Monitoring System (IMS) is a verification component of the Comprehensive Nuclear-Test-Ban Treaty (CTBT), and in addition to a series of radionuclide monitoring stations, contains sixteen radionuclide laboratories capable of verification of radionuclide station measurements. This paper presents an overview of a new commercially obtained low-background detector system for radionuclide aerosol measurements recently installed in a shallow (>30 meters water equivalent) underground clean-room facility at Pacific Northwest National Laboratory. Specifics such as low-background shielding materials, active shielding methods, and improvements in sensitivity to IMS isotopes will be covered.

  2. Geant4 simulation of continuum gamma spectroscopy with GAMMASPHERE and the SPINSPECTROMETER

    SciTech Connect

    Silva, Z.; Ferrer, M.; Cristancho, F.

    2007-10-26

    The use of the so called Hk-technique ({gamma}-energy sum and multiplicity data) is checked with simulations of the multi-detector {gamma}-arrays GAMMASPHERE and SPINSPECTROMETER. Their response to typical {gamma}-cascades is obtained and compared.

  3. Structure of the propeptide of prothrombin containing the. gamma. -carboxylation recognition site determined by two-dimensional NMR spectroscopy

    SciTech Connect

    Sanford, D.G.; Sudmeier, J.L.; Bachovchin, W.W.; Kanagy, C.; Furie, B.C.; Furie, B. )

    1991-10-15

    The propeptides of the vitamin K dependent blood clotting and regulatory proteins contain a {gamma}-carboxylation recognition site that directs precursor forms of these proteins for posttranslational {gamma}-carboxylation. Peptides corresponding to the propeptide of prothrombin were synthesized and examined by circular dichroism (CD) and nuclear magnetic resonance spectroscopy (NMR). CD spectra indicate that these peptides have little or no secondary structure in aqueous solutions but that the addition of trifluoroethanol induces or stabilizes a structure containing {alpha}-helical character. The maximum helical content occurs at 35-40% trifluoroethanol. This trifluoroethanol-stabilized structure was solved by two-dimensional NMR spectroscopy. The NMR results demonstrate that residues {minus}13 to {minus}3 form an amphipathic {alpha}-helix. NMR spectra indicate that a similar structure is present at 5C, in the absence of trifluoroethanol. Of the residues previously implicated in defining the {gamma}-carboxylation recognition site, four residues ({minus}18, {minus}17, {minus}16, and {minus}15) are adjacent to the helical region and one residue ({minus}10) is located within the helix. The potential role of the amphipathic {alpha}-helix in the {gamma}-carboxylation recognition site is discussed.

  4. Structure of the propeptide of prothrombin containing the gamma-carboxylation recognition site determined by two-dimensional NMR spectroscopy.

    PubMed

    Sanford, D G; Kanagy, C; Sudmeier, J L; Furie, B C; Furie, B; Bachovchin, W W

    1991-10-15

    The propeptides of the vitamin K dependent blood clotting and regulatory proteins contain a gamma-carboxylation recognition site that directs precursor forms of these proteins for posttranslational gamma-carboxylation. Peptides corresponding to the propeptide of prothrombin were synthesized and examined by circular dichroism (CD) and nuclear magnetic resonance spectroscopy (NMR). CD spectra indicate that these peptides have little or no secondary structure in aqueous solutions but that the addition of trifluoroethanol induces or stabilizes a structure containing alpha-helical character. The maximum helical content occurs at 35-40% trifluoroethanol. This trifluoroethanol-stabilized structure was solved by two-dimensional NMR spectroscopy. The NMR results demonstrate that residues -13 to -3 form an amphipathic alpha-helix. NMR spectra indicate that a similar structure is present at 5 degrees C, in the absence of trifluoroethanol. Of the residues previously implicated in defining the gamma-carboxylation recognition site, four residues (-18, -17, -16, and -15) are adjacent to the helical region and one residue (-10) is located within the helix. The potential role of the amphipathic alpha-helix in the gamma-carboxylation recognition site is discussed. PMID:1911775

  5. Conformational solution studies of neuropeptide gamma using CD and NMR spectroscopy.

    PubMed

    Rodziewicz-Motowidło, Sylwia; Brzozowskl, Krzysztof; Legowska, Anna; Liwo, Adam; Silbering, Jerzy; Smoluch, Marek; Rolka, Krzysztof

    2002-05-01

    Neuropeptide gamma is one of the largest members of the tachykinin family of peptides, exhibiting strong agonistic activity towards the NK-2 tachykinin receptor. This peptide was synthesized by the solid-phase method using the Fmoc chemistry. Circular-dichroism spectroscopy (CD) investigations of this peptide were performed in phosphate buffer, in the presence of sodium dodecylsulphate (SDS) micelles and trifluoroethanol (TFE) solutions and in DMSO-d6 using the 2D NMR technique in conjunction with two different theoretical approaches. The first assumes multiconformational equilibrium of the peptide studied characterized by the values of statistical weights of low-energy conformations. These calculations were performed using three different force fields ECEPP/3, AMBER4.1 and CHARMM (implemented in the X-PLOR program). The second method incorporates interproton distance and dihedral angle constraints into the starting conformation using the Simulated Annealing algorithm (X-PLOR program). The CD experiments revealed that although the peptide studied is flexible in polar solvents, a tendency to adopt a helical structure was observed in the hydrophobic environment. The NMR data (NOE effects) indicate a helical or reverse structure in the Ile7-His12 fragment of the peptide studied in DMSO-d6 solution. The results obtained cannot be interpreted in terms of a single conformation. Most of the conformations obtained with the ECEPP/3 force field possess a high content of a helical structure. None of the conformers, obtained with the AMBER4.1 and CHARMM force fields, can be considered as the dominant one. In all conformations several beta-turns were detected and in some cases gamma-turns were also found. But in fact, it is rather difficult to select the position of the secondary element(s) present in the structure of NPgamma in solution. All conformers calculated with the X-PLOR program (with using NMR derived distance and torsion angle constraints) are stabilized by several

  6. Investigation of Martian H2O and CO2 via orbital gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Evans, Larry G.; Squyres, Steven W.

    1987-01-01

    The capability of an orbital gamma ray spectrometer to address presently unanswered questions concerning H2O and CO2 on Mars is investigated. The gamma ray signal produced by the Martian atmosphere and by several simple models of Martian surface materials is calculated. Results are reported for: (1) the production of neutrons in the atmosphere and in the subsurface material by cosmic ray interactions, (2) the scattering of neutrons and the resultant neutron energy spectrum and spatial distributions, (3) the reproduction of gamma rays by neutron prompt capture and nonelastic scatter reactions, (4) the production of gamma rays by natural radionuclides, (5) the attenuation of the gamma ray signal by passage through surface materials and the Martian atmosphere, (6) the production of the gamma ray continuum background, and (7) the uncertainty in gamma ray line strengths that results from the combined signal and background observed by the detector.

  7. Investigation of Martian H2O and CO2 via orbital gamma ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Evans, L. G.; Squyres, S. W.

    1987-08-01

    The capability of an orbital gamma ray spectrometer to address presently unanswered questions concerning H2O and CO2 on Mars is investigated. The gamma ray signal produced by the Martian atmosphere and by several simple models of Martian surface materials is calculated. Results are reported for: (1) the production of neutrons in the atmosphere and in the subsurface material by cosmic ray interactions, (2) the scattering of neutrons and the resultant neutron energy spectrum and spatial distributions, (3) the reproduction of gamma rays by neutron prompt capture and nonelastic scatter reactions, (4) the production of gamma rays by natural radionuclides, (5) the attenuation of the gamma ray signal by passage through surface materials and the Martian atmosphere, (6) the production of the gamma ray continuum background, and (7) the uncertainty in gamma ray line strengths that results from the combined signal and background observed by the detector.

  8. Astroparticle physics with a customized low-background broad energy Germanium detector

    NASA Astrophysics Data System (ADS)

    Aalseth, C. E.; Amman, M.; Avignone, F. T.; Back, H. O.; Barabash, A. S.; Barbeau, P. S.; Bergevin, M.; Bertrand, F. E.; Boswell, M.; Brudanin, V.; Bugg, W.; Burritt, T. H.; Busch, M.; Capps, G.; Chan, Y.-D.; Collar, J. I.; Cooper, R. J.; Creswick, R.; Detwiler, J. A.; Diaz, J.; Doe, P. J.; Efremenko, Yu.; Egorov, V.; Ejiri, H.; Elliott, S. R.; Ely, J.; Esterline, J.; Farach, H.; Fast, J. E.; Fields, N.; Finnerty, P.; Fujikawa, B.; Fuller, E.; Gehman, V. M.; Giovanetti, G. K.; Guiseppe, V. E.; Gusey, K.; Hallin, A. L.; Harper, G. C.; Hazama, R.; Henning, R.; Hime, A.; Hoppe, E. W.; Hossbach, T. W.; Howe, M. A.; Johnson, R. A.; Keeter, K. J.; Keillor, M.; Keller, C.; Kephart, J. D.; Kidd, M. F.; Knecht, A.; Kochetov, O.; Konovalov, S. I.; Kouzes, R. T.; Leviner, L.; Loach, J. C.; Luke, P. N.; Macmullin, S.; Marino, M. G.; Martin, R. D.; Mei, D.-M.; Miley, H. S.; Miller, M. L.; Mizouni, L.; Meyers, A. W.; Nomachi, M.; Orrell, J. L.; Peterson, D.; Phillips, D. G.; Poon, A. W. P.; Prior, G.; Qian, J.; Radford, D. C.; Rielage, K.; Robertson, R. G. H.; Rodriguez, L.; Rykaczewski, K. P.; Salazar, H.; Schubert, A. G.; Shima, T.; Shirchenko, M.; Steele, D.; Strain, J.; Swift, G.; Thomas, K.; Timkin, V.; Tornow, W.; van Wechel, T. D.; Vanyushin, I.; Varner, R. L.; Vetter, K.; Wilkerson, J. F.; Wolfe, B. A.; Xiang, W.; Yakushev, E.; Yaver, H.; Young, A. R.; Yu, C.-H.; Yumatov, V.; Zhang, C.; Zimmerman, S.; M Ajorana Collaboration

    2011-10-01

    The MAJORANA Collaboration is building the MAJORANA DEMONSTRATOR, a 60 kg array of high purity germanium detectors housed in an ultra-low background shield at the Sanford Underground Laboratory in Lead, SD. The MAJORANA DEMONSTRATOR will search for neutrinoless double-beta decay of 76Ge while demonstrating the feasibility of a tonne-scale experiment. It may also carry out a dark matter search in the 1-10 GeV/ c2 mass range. We have found that customized Broad Energy Germanium (BEGe) detectors produced by Canberra have several desirable features for a neutrinoless double-beta decay experiment, including low electronic noise, excellent pulse shape analysis capabilities, and simple fabrication. We have deployed a customized BEGe, the MAJORANA Low-Background BEGe at Kimballton (MALBEK), in a low-background cryostat and shield at the Kimballton Underground Research Facility in Virginia. This paper will focus on the detector characteristics and measurements that can be performed with such a radiation detector in a low-background environment.

  9. Astroparticle physics with a customized low-background broad energy Germanium detector

    SciTech Connect

    Aalseth, Craig E.; Amman, M.; Avignone, Frank T.; Back, Henning O.; Barabash, Alexander S.; Barbeau, P. S.; Bergevin, M.; Bertrand, F.; Boswell, M.; Brudanin, V.; Bugg, William; Burritt, Tom H.; Busch, Matthew; Capps, Greg L.; Chan, Yuen-Dat; Collar, J. I.; Cooper, R. J.; Creswick, R.; Detwiler, Jason A.; Diaz, J.; Doe, Peter J.; Efremenko, Yuri; Egorov, Viatcheslav; Ejiri, H.; Elliott, Steven R.; Ely, James H.; Esterline, James H.; Farach, H. A.; Fast, James E.; Fields, N.; Finnerty, P.; Fujikawa, Brian; Fuller, Erin S.; Gehman, Victor M.; Giovanetti, G. K.; Guiseppe, Vincente; Gusey, K.; Hallin, A. L.; Harper, Gregory; Hazama, R.; Henning, Reyco; Hime, Andrew; Hoppe, Eric W.; Hossbach, Todd W.; Howe, M. A.; Johnson, R. A.; Keeter, K.; Keillor, Martin E.; Keller, C.; Kephart, Jeremy D.; Kidd, Mary; Knecht, A.; Kochetov, Oleg; Konovalov, S.; Kouzes, Richard T.; Leviner, L.; Loach, J. C.; Luke, P.; MacMullin, S.; Marino, Michael G.; Martin, R. D.; Mei, Dong-Ming; Miley, Harry S.; Miller, M. L.; Mizouni, Leila; Myers, Allan W.; Nomachi, Masaharu; Orrell, John L.; Peterson, David; Phillips, D.; Poon, Alan; Prior, Gersende; Qian, J.; Radford, D. C.; Rielage, Keith; Robertson, R. G. H.; Rodriguez, Larry; Rykaczewski, Krzysztof P.; Salazar, Harold; Schubert, Alexis G.; Shima, T.; Shirchenko, M.; Steele, David; Strain, J.; Swift, Gary; Thomas, K.; Timkin, V.; Tornow, W.; Van Wechel, T. D.; Vanyushin, I.; Varner, R. L.; Vetter, Kai; Wilkerson, J. F.; Wolfe, B. A.; Xiang, W.; Yakushev, E.; Yaver, Harold; Young, A.; Yu, Chang-Hong; Yumatov, Vladimir; Zhang, C.; Zimmerman, S.

    2011-10-01

    The Majorana Collaboration is building the Majorana Demonstrator, a 60 kg array of high purity germanium detectors housed in an ultra-low background shield at the Sanford Underground Laboratory in Lead, SD. The Majorana Demonstrator will search for neutrinoless double-beta decay of 76Ge while demonstrating the feasibility of a tonne-scale experiment. It may also carry out a dark matter search in the 1-10 GeV/c² mass range. We have found that customized Broad Energy Germanium (BEGe) detectors produced by Canberra have several desirable features for a neutrinoless double-beta decay experiment, including low electronic noise, excellent pulse shape analysis capabilities, and simple fabrication. We have deployed a customized BEGe, the Majorana Low-Background BEGe at Kimballton (MALBEK), in a low-background cryostat and shield at the Kimballton Underground Research Facility in Virginia. This paper will focus on the detector characteristics and measurements that can be performed with such a radiation detector in a low-background environment.

  10. Development of a Small-Sized, Flexible, and Insertable Fiber-Optic Radiation Sensor for Gamma-Ray Spectroscopy

    PubMed Central

    Yoo, Wook Jae; Shin, Sang Hun; Lee, Dong Eun; Jang, Kyoung Won; Cho, Seunghyun; Lee, Bongsoo

    2015-01-01

    We fabricated a small-sized, flexible, and insertable fiber-optic radiation sensor (FORS) that is composed of a sensing probe, a plastic optical fiber (POF), a photomultiplier tube (PMT)-amplifier system, and a multichannel analyzer (MCA) to obtain the energy spectra of radioactive isotopes. As an inorganic scintillator for gamma-ray spectroscopy, a cerium-doped lutetium yttrium orthosilicate (LYSO:Ce) crystal was used and two solid-disc type radioactive isotopes with the same dimensions, cesium-137 (Cs-137) and cobalt-60 (Co-60), were used as gamma-ray emitters. We first determined the length of the LYSO:Ce crystal considering the absorption of charged particle energy and measured the gamma-ray energy spectra using the FORS. The experimental results demonstrated that the proposed FORS can be used to discriminate species of radioactive isotopes by measuring their inherent energy spectra, even when gamma-ray emitters are mixed. The relationship between the measured photon counts of the FORS and the radioactivity of Cs-137 was subsequently obtained. The amount of scintillating light generated from the FORS increased by increasing the radioactivity of Cs-137. Finally, the performance of the fabricated FORS according to the length and diameter of the POF was also evaluated. Based on the results of this study, it is anticipated that a novel FORS can be developed to accurately measure the gamma-ray energy spectrum in inaccessible locations such as narrow areas and holes. PMID:26343667

  11. Development of a Small-Sized, Flexible, and Insertable Fiber-Optic Radiation Sensor for Gamma-Ray Spectroscopy.

    PubMed

    Yoo, Wook Jae; Shin, Sang Hun; Lee, Dong Eun; Jang, Kyoung Won; Cho, Seunghyun; Lee, Bongsoo

    2015-01-01

    We fabricated a small-sized, flexible, and insertable fiber-optic radiation sensor (FORS) that is composed of a sensing probe, a plastic optical fiber (POF), a photomultiplier tube (PMT)-amplifier system, and a multichannel analyzer (MCA) to obtain the energy spectra of radioactive isotopes. As an inorganic scintillator for gamma-ray spectroscopy, a cerium-doped lutetium yttrium orthosilicate (LYSO:Ce) crystal was used and two solid-disc type radioactive isotopes with the same dimensions, cesium-137 (Cs-137) and cobalt-60 (Co-60), were used as gamma-ray emitters. We first determined the length of the LYSO:Ce crystal considering the absorption of charged particle energy and measured the gamma-ray energy spectra using the FORS. The experimental results demonstrated that the proposed FORS can be used to discriminate species of radioactive isotopes by measuring their inherent energy spectra, even when gamma-ray emitters are mixed. The relationship between the measured photon counts of the FORS and the radioactivity of Cs-137 was subsequently obtained. The amount of scintillating light generated from the FORS increased by increasing the radioactivity of Cs-137. Finally, the performance of the fabricated FORS according to the length and diameter of the POF was also evaluated. Based on the results of this study, it is anticipated that a novel FORS can be developed to accurately measure the gamma-ray energy spectrum in inaccessible locations such as narrow areas and holes. PMID:26343667

  12. The BATSE Gamma-Ray Burst Spectral Catalog. 1; High Time Resolution Spectroscopy of Bright Bursts Using High Energy Resolution Data

    NASA Technical Reports Server (NTRS)

    Preece, Robert D.; Briggs, Michael S.; Mallozzi, Robert S.; Pendleton, Geoffrey N.; Paciesas, W. S.; Band, David L.

    1999-01-01

    This is the first in a series of gamma-ray burst spectroscopy catalogs from the Burst And Transient Source Experiment (BATSE) on the Compton Gamma Ray Abstract: Observatory, each covering a different aspect of burst phenomenology. In this paper, we present time-sequences of spectral fit parameters for 156 bursts selected either for their high peak flux or fluence.

  13. ACTI - An MCNP Data Library for Prompt Gamma-Ray Spectroscopy.

    SciTech Connect

    Frankle, S. C.; Reedy, R. C.; Young, P. G. ,

    2002-01-01

    Prompt gamma-ray spectroscopy is used in a wide variety of applications for determining material compositions. High-quality photon-production data from thermal-neutron capture reactions are essential for these applications. Radiation transport codes, such as MCNP{trademark}, are often used to design detector systems, determine minimum detection thresholds, etc. These transport codes rely on evaluated nuclear databases such as ENDF (Evaluated Nuclear Data File) to provide the fundamental data used in the transport calculations. Often the photon-production data from incident neutron reactions in the evaluations are of relatively poor quality. We have compiled the best experimental data for thermal-neutron capture for the naturally occurring isotopes for elements from H through Zn as well as for {sup 70,72,73,74,76}Ge, {sup 149}Sm, {sup 155,157}Gd, {sup 181}Ta and {sup 182,183,184,186}W. This compilation has been used to update the ENDF evaluations for {sup 1}H, {sup 4}He, {sup 9}Be, {sup 14}N, {sup 16}O, {sup 19}F, Na, Mg, {sup 27}Al, {sup 32}S, S, {sup 35,37}Cl, K, Ca, {sup 45}Sc, Ti, {sup 51}V, {sup 50,52,53,54}Cr, {sup 55}Mn, {sup 54,56,57,58}Fe, {sup 58,60,61,62,64}Ni, {sup 63,65}Cu and {sup 182,183,184,186}W. In addition, the inelastic cross sections and corresponding secondary-photon distributions were updated for {sup 16}O. Complete new evaluations were submitted to ENDF for {sup 35,37}Cl. This paper will discuss the evaluation effort and the production of the MCNP data library, ACTI, based on the new evaluations. Data from the ENDF evaluations for {sup 28-30}Si were also included in the ACTI library for completeness. The silicon evaluations were updated in 1997 and include the latest experimental data for radiative capture.

  14. Proximal Gamma-Ray Spectroscopy to Predict Soil Properties Using Windows and Full-Spectrum Analysis Methods

    PubMed Central

    Mahmood, Hafiz Sultan; Hoogmoed, Willem B.; van Henten, Eldert J.

    2013-01-01

    Fine-scale spatial information on soil properties is needed to successfully implement precision agriculture. Proximal gamma-ray spectroscopy has recently emerged as a promising tool to collect fine-scale soil information. The objective of this study was to evaluate a proximal gamma-ray spectrometer to predict several soil properties using energy-windows and full-spectrum analysis methods in two differently managed sandy loam fields: conventional and organic. In the conventional field, both methods predicted clay, pH and total nitrogen with a good accuracy (R2 ≥ 0.56) in the top 0–15 cm soil depth, whereas in the organic field, only clay content was predicted with such accuracy. The highest prediction accuracy was found for total nitrogen (R2 = 0.75) in the conventional field in the energy-windows method. Predictions were better in the top 0–15 cm soil depths than in the 15–30 cm soil depths for individual and combined fields. This implies that gamma-ray spectroscopy can generally benefit soil characterisation for annual crops where the condition of the seedbed is important. Small differences in soil structure (conventional vs. organic) cannot be determined. As for the methodology, we conclude that the energy-windows method can establish relations between radionuclide data and soil properties as accurate as the full-spectrum analysis method. PMID:24287541

  15. Gamma-ray burst spectroscopy capabilities of the BATSE/GRO experiment

    NASA Technical Reports Server (NTRS)

    Matteson, J. L.; Fishman, G. J.; Meegan, C. A.; Parnell, T. A.; Wilson, R. B.; Paciesas, W.; Cline, T. L.; Teegarden, B. J.

    1985-01-01

    A scintillation spectrometer is included in each of the eight BATSE/GRO detector modules, resulting in all-sky coverage for gamma-ray bursts. The scientific motivation, design and capabilities of these spectrometers for performing spectral observations over a wide range of gamma-ray energies and burst intensities are described.

  16. Gator: a low-background counting facility at the Gran Sasso Underground Laboratory

    NASA Astrophysics Data System (ADS)

    Baudis, L.; Ferella, A. D.; Askin, A.; Angle, J.; Aprile, E.; Bruch, T.; Kish, A.; Laubenstein, M.; Manalaysay, A.; Marrodán Undagoitia, T.; Schumann, M.

    2011-08-01

    A low-background germanium spectrometer has been installed and is being operated in an ultra-low background shield (the Gator facility) at the Gran Sasso underground laboratory in Italy (LNGS). With an integrated rate of ~ 0.16 events/min in the energy range between 100-2700 keV, the background is comparable to those of the world's most sensitive germanium detectors. After a detailed description of the facility, its background sources as well as the calibration and efficiency measurements are introduced. Two independent analysis methods are described and compared using examples from selected sample measurements. The Gator facility is used to screen materials for XENON, GERDA, and in the context of next-generation astroparticle physics facilities such as DARWIN.

  17. Real time method and computer system for identifying radioactive materials from HPGe gamma-ray spectroscopy

    DOEpatents

    Rowland, Mark S.; Howard, Douglas E.; Wong, James L.; Jessup, James L.; Bianchini, Greg M.; Miller, Wayne O.

    2007-10-23

    A real-time method and computer system for identifying radioactive materials which collects gamma count rates from a HPGe gamma-radiation detector to produce a high-resolution gamma-ray energy spectrum. A library of nuclear material definitions ("library definitions") is provided, with each uniquely associated with a nuclide or isotope material and each comprising at least one logic condition associated with a spectral parameter of a gamma-ray energy spectrum. The method determines whether the spectral parameters of said high-resolution gamma-ray energy spectrum satisfy all the logic conditions of any one of the library definitions, and subsequently uniquely identifies the material type as that nuclide or isotope material associated with the satisfied library definition. The method is iteratively repeated to update the spectrum and identification in real time.

  18. New concepts for HgI2 scintillator gamma ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Iwanczyk, Jan S.

    1994-01-01

    The primary goals of this project are development of the technology for HgI2 photodetectors (PD's), development of a HgI2/scintillator gamma detector, development of electronics, and development of a prototype gamma spectrometer. Work on the HgI2 PD's involved HgI2 purification and crystal growth, detector surface and electrical contact studies, PD structure optimization, encapsulation and packaging, and testing. Work on the HgI2/scintillator gamma detector involved a study of the optical - mechanical coupling for the optimization of CsI(Tl)/HgI2 gamma ray detectors and determination of the relationship between resolution versus scintillator type and size. The development of the electronics focused on low noise amplification circuits using different preamp input FET's and the use of a coincidence technique to maximize the signal, minimize the noise contribution in the gamma spectra, and improve the overall system resolution.

  19. The low background spectrometer TGV II for double beta decay measurements

    NASA Astrophysics Data System (ADS)

    Beneš, P.; Čermák, P.; Gusev, K. N.; Klimenko, A. A.; Kovalenko, V. E.; Kovalík, A.; Rukhadze, N. I.; Salamatin, A. V.; Šimkovic, F.; Štekl, I.; Timkin, V. V.; Vylov, Ts.

    2006-12-01

    The low-background multi-HPGe spectrometer TGV II installed in the Modane Underground Laboratory (France) is described in detail and the results of the background measurements are reported. The spectrometer is focused on the double beta decay measurements with two isotopes— 106Cd ( 2νEC/EC mode) and 48Ca ( ββ mode). A basic summary of the physics of ββ decay (especially EC/EC mode) is also given.

  20. Development of optimized detector/spectrophotometer technology for low background space astronomy missions

    NASA Technical Reports Server (NTRS)

    Jones, B.

    1985-01-01

    This program was directed towards a better understanding of some of the important factors in the performance of infrared detector arrays at low background conditions appropriate for space astronomy. The arrays were manufactured by Aerojet Electrosystems Corporation, Azusa. Two arrays, both bismuth doped silicon, were investigated: an AMCID 32x32 Engineering mosiac Si:Bi accumulation mode charge injection device detector array and a metal oxide semiconductor/field effect transistor (MOS-FET) switched array of 16x32 pixels.

  1. Assessment study of infrared detector arrays for low-background astronomical research

    NASA Technical Reports Server (NTRS)

    Ando, K. J.

    1978-01-01

    The current state-of-the-art of infrared detector arrays employing charge coupled devices (CCD) or charge injection devices (CID) readout are assessed. The applicability, limitations and potentials of such arrays under the low-background astronomical observing conditions of interest for SIRFT (Shuttle Infrared Telescope Facility) are determined. The following are reviewed: (1) monolithic extrinsic arrays; (2) monolithic intrinsic arrays; (3) charge injection devices; and (4) hybrid arrays.

  2. Evaluation of ultra-low background materials for uranium and thorium using ICP-MS

    SciTech Connect

    Hoppe, E. W.; Overman, N. R.; LaFerriere, B. D.

    2013-08-08

    An increasing number of physics experiments require low background materials for their construction. The presence of Uranium and Thorium and their progeny in these materials present a variety of unwanted background sources for these experiments. The sensitivity of the experiments continues to drive the necessary levels of detection ever lower as well. This requirement for greater sensitivity has rendered direct radioassay impractical in many cases requiring large quantities of material, frequently many kilograms, and prolonged counting times, often months. Other assay techniques have been employed such as Neutron Activation Analysis but this requires access to expensive facilities and instrumentation and can be further complicated and delayed by the formation of unwanted radionuclides. Inductively Coupled Plasma Mass Spectrometry (ICP-MS) is a useful tool and recent advancements have increased the sensitivity particularly in the elemental high mass range of U and Th. Unlike direct radioassay, ICP-MS is a destructive technique since it requires the sample to be in liquid form which is aspirated into a high temperature plasma. But it benefits in that it usually requires a very small sample, typically about a gram. This paper discusses how a variety of low background materials such as copper, polymers, and fused silica are made amenable to ICP-MS assay and how the arduous task of maintaining low backgrounds of U and Th is achieved.

  3. DESIGN OF A THERMOSIPHON FOR COOLING LOW-BACKGROUND HPGE ARRAYS

    SciTech Connect

    Aguayo Navarrete, Estanislao; Fast, James E.; Reid, Douglas J.

    2012-11-26

    ABSTRACT A two-phase nitrogen thermosiphon was developed for the new generation of low-background high-purity germanium (HPGe) arrays. The cooling system for these arrays has to be able to handle the heat load (>20 W) presented by a large detector mass while meeting stringent requirements necessary for low-background systems. The HPGe detector modules should operate as close to liquid nitrogen temperature (<80K) as possible to provide adequate operating conditions for a full range of HPGe impurity concentrations. In addition, exceptional temperature stability (<1 K) is needed to reduce electronic gain shifts due to changes in the front-end electronics operating temperature. In order to meet the background requirements of state-of-the-art systems these arrays are enclosed in passive lead and copper shielding up to 1 m thick. In this paper we present a cooling system for low-background experiments that complies with these stringent geometrical restrictions. Active cooling was integrated via a horizontal thermosiphon that can be fabricated using ultra-pure electroformed copper. It was charged with nitrogen to 434 kPa (63 PSIA) at 292 K, which provided a fill ratio of 10%. The results showed that the thermosiphon can effectively remove in excess of 25 W of heat load.

  4. Evaluation of ultra-low background materials for uranium and thorium using ICP-MS

    NASA Astrophysics Data System (ADS)

    Hoppe, E. W.; Overman, N. R.; LaFerriere, B. D.

    2013-08-01

    An increasing number of physics experiments require low background materials for their construction. The presence of Uranium and Thorium and their progeny in these materials present a variety of unwanted background sources for these experiments. The sensitivity of the experiments continues to drive the necessary levels of detection ever lower as well. This requirement for greater sensitivity has rendered direct radioassay impractical in many cases requiring large quantities of material, frequently many kilograms, and prolonged counting times, often months. Other assay techniques have been employed such as Neutron Activation Analysis but this requires access to expensive facilities and instrumentation and can be further complicated and delayed by the formation of unwanted radionuclides. Inductively Coupled Plasma Mass Spectrometry (ICP-MS) is a useful tool and recent advancements have increased the sensitivity particularly in the elemental high mass range of U and Th. Unlike direct radioassay, ICP-MS is a destructive technique since it requires the sample to be in liquid form which is aspirated into a high temperature plasma. But it benefits in that it usually requires a very small sample, typically about a gram. This paper discusses how a variety of low background materials such as copper, polymers, and fused silica are made amenable to ICP-MS assay and how the arduous task of maintaining low backgrounds of U and Th is achieved.

  5. Evaluation of Ultra-Low Background Materials for Uranium and Thorium Using ICP-MS

    SciTech Connect

    Hoppe, Eric W.; Overman, Nicole R.; LaFerriere, Brian D.

    2013-08-08

    An increasing number of physics experiments require low background materials for their construction. The presence of Uranium and Thorium and their progeny in these materials present a variety of unwanted background sources for these experiments. The sensitivity of the experiments continues to drive the necessary levels of detection ever lower as well. This requirement for greater sensitivity has rendered direct radioassay impractical in many cases requiring large quantities of material, frequently many kilograms, and prolonged counting times, often months. Other assay techniques have been employed such as Neutron Activation Analysis but this requires access to expensive facilities and instrumentation and can be further complicated and delayed by the formation of unwanted radionuclides. Inductively Coupled Plasma Mass Spectrometry (ICP-MS) is a useful tool and recent advancements have increased the sensitivity particularly in the elemental high mass range of U and Th. Unlike direct radioassay, ICP-MS is a destructive technique since it requires the sample to be in liquid form which is aspirated into a high temperature plasma. But it benefits in that it usually requires a very small sample, typically about a gram. Here we will discuss how a variety of low background materials such as copper, polymers, and fused silica are made amenable to ICP-MS assay and how the arduous task of maintaining low backgrounds of U and Th is achieved.

  6. Feasibility on the spectrometric determination of the individual dose rate for detected gamma nuclides using the dose rate spectroscopy

    NASA Astrophysics Data System (ADS)

    Ji, Young-Yong; Chung, Kun Ho; Lee, Wanno; Park, Doo-Won; Kang, Mun-Ja

    2014-04-01

    A spectrometric determination of the dose rate using a detector is a very useful method to identify the contribution of artificial nuclides. In addition, the individual dose rate for detected gamma nuclides from the radioactive materials as well as the environment can give further information such as the in-situ measurement because of the direct relation between the individual dose rate and the activity of a nuclide. In this study, the calculation method for the individual dose rate for detected gamma nuclides was suggested by introducing the concept of the dose rate spectroscopy and the peak-to-total ratio in the energy spectrum for the dose rate, which means just a form of multiplied counts and the value of a G-factor in the spectrum. In addition, the validity of the suggested method for the individual dose rate was experimentally verified through a comparison of the calculation results on the energy spectra for several conditions of the standard source.

  7. Lu1-xI3:Cex--A Scintillator for gamma ray spectroscopy and time-of-flight PET

    DOEpatents

    Shah, Kanai S.

    2009-03-17

    The present invention concerns very fast scintillator materials comprising lutetium iodide doped with Cerium Lu.sub.1-xI.sub.3:Ce.sub.x; LuI.sub.3:Ce). The LuI.sub.3 scintillator material has surprisingly good characteristics including high light output, high gamma ray stopping efficiency, fast response, low cost, good proportionality, and minimal afterglow that the material is useful for gamma ray spectroscopy, medical imaging, nuclear and high energy physics research, diffraction, non-destructive testing, nuclear treaty verification and safeguards, and geological exploration. The timing resolution of the scintillators of the present invention provide compositions capable of resolving the position of an annihilation event within a portion of a human body cross-section.

  8. A novel liquid-Xenon detector concept for combined fast-neutrons and gamma imaging and spectroscopy

    NASA Astrophysics Data System (ADS)

    Breskin, A.; Israelashvili, I.; Cortesi, M.; Arazi, L.; Shchemelinin, S.; Chechik, R.; Dangendorf, V.; Bromberger, B.; Vartsky, D.

    2012-06-01

    A new detector concept is presented for combined imaging and spectroscopy of fast-neutrons and gamma rays. It comprises a liquid-Xenon (LXe) converter and scintillator coupled to a UV-sensitive gaseous imaging photomultiplier (GPM). Radiation imaging is obtained by localization of the scintillation-light from LXe with the position-sensitive GPM. The latter comprises a cascade of Thick Gas Electron Multipliers (THGEM), where the first element is coated with a CsI UV-photocathode. We present the concept and provide first model-simulation results of the processes involved and the expected performances of a detector having a LXe-filled capillaries converter. The new detector concept has potential applications in combined fast-neutron and gamma-ray screening of hidden explosives and fissile materials with pulsed sources.

  9. Low-background shielding of Ge detectors for the measurement of residual 152Eu radioactivity induced by neutrons from the Hiroshima atomic bomb

    NASA Astrophysics Data System (ADS)

    Shizuma, Kiyoshi; Fukami, Kenji; Iwatani, Kazuo; Hasai, Hiromi

    1992-05-01

    Low-background gamma-ray spectrometers were constructed for the measurement of residual 152Eu activity induced by the atomic-bomb neutrons. Optimum thickness of lead shielding, inner linings and background characteristics were investigated for an ordinary coaxial- and a well-type Ge detector. In addition, an anticoincidence shielding was installed for the well-type detector. As a result, the background counting rate due to cosmic rays was greatly reduced. It was also shown that a sample preparation to enrich the objective activity and eliminate background activities was important in the case of the 152Eu measurement.

  10. POSITION SENSITIVE GERMANIUM DETECTORS FOR GAMMA-RAY IMAGING AND SPECTROSCOPY

    EPA Science Inventory

    Gamma-ray imaging with position-sensitive germanium detectors offers the advantages of excellent energy resolution, high detection efficiency, and potentially good sptial resolution. The development of the amorphous-semiconductor electrical contact technology for germanium detec...

  11. Detection system for high-resolution gamma radiation spectroscopy with neutron time-of-flight filtering

    DOEpatents

    Dioszegi, Istvan; Salwen, Cynthia; Vanier, Peter

    2014-12-30

    A .gamma.-radiation detection system that includes at least one semiconductor detector such as HPGe-Detector, a position-sensitive .alpha.-Detector, a TOF Controller, and a Digitizer/Integrator. The Digitizer/Integrator starts to process the energy signals of a .gamma.-radiation sent from the HPGe-Detector instantly when the HPGe-Detector detects the .gamma.-radiation. Subsequently, it is determined whether a coincidence exists between the .alpha.-particles and .gamma.-radiation signal, based on a determination of the time-of-flight of neutrons obtained from the .alpha.-Detector and the HPGe-Detector. If it is determined that the time-of-flight falls within a predetermined coincidence window, the Digitizer/Integrator is allowed to continue and complete the energy signal processing. If, however, there is no coincidence, the Digitizer/Integrator is instructed to be clear and reset its operation instantly.

  12. Prompt {gamma}-ray spectroscopy of the {sup 104}Mo and {sup 108}Mo fission fragments

    SciTech Connect

    Guessous, A.; Schulz, N.; Bentaleb, M.; Lubkiewicz, E.; Durell, J.L.; Pearson, C.J.; Phillips, W.R.; Shannon, J.A.; Urban, W.; Varley, B.J.; Ahmad, I.; Lister, C.J.; Morss, L.R.; Nash, K.L.; Williams, C.W.; Khazrouni, S.

    1996-03-01

    The level structures of the neutron-rich {sup 104}Mo and {sup 108}Mo nuclei have been investigated by observing prompt {gamma} rays emitted in the spontaneous fission of {sup 248}Cm with the EUROGAM spectrometer. Levels with spins up to 12{h_bar} have been observed and {gamma} branching obtained. The data can be satisfactorily described when {sup 104,108}Mo are considered as axially symmetric nuclei: in {sup 104}Mo, rotational bands based on the ground state, the one-phonon and the two-phonon {gamma}-vibrational states and a quasiparticle state have been observed, whereas in {sup 108}Mo the information is limited to the yrast band and the one phonon {gamma} band. {copyright} {ital 1996 The American Physical Society.}

  13. {gamma}-Spectroscopy and Radioactive Beams: How To Perform Channel Selection ?

    SciTech Connect

    Rosse, B.; Redon, N.; Stezowski, O.; Schmitt, Ch.; Guinet, D.; Meyer, M.; Lautesse, Ph.; De France, G.; Bhattachasyya, S.; Mukherjee, G.

    2006-04-26

    An experiment has been performed using a SPIRAL 76Kr radioactive beam at GANIL to investigate rare-earth nuclei near the proton drip-line. The EXOGAM gamma array was coupled with the DIAMANT light charged-particle detector and the VAMOS spectrometer. We report here on the powerful of this setup to extract fusion-evaporation {gamma}-rays from a large beam contamination.

  14. Time-resolved Spectroscopy of the Three Brightest and Hardest Short Gamma-ray Bursts Observed with the Fermi Gamma-ray Burst Monitor

    NASA Astrophysics Data System (ADS)

    Guiriec, Sylvain; Briggs, Michael S.; Connaugthon, Valerie; Kara, Erin; Daigne, Frédéric; Kouveliotou, Chryssa; van der Horst, Alexander J.; Paciesas, William; Meegan, Charles A.; Bhat, P. N.; Foley, Suzanne; Bissaldi, Elisabetta; Burgess, Michael; Chaplin, Vandiver; Diehl, Roland; Fishman, Gerald; Gibby, Melissa; Giles, Misty M.; Goldstein, Adam; Greiner, Jochen; Gruber, David; von Kienlin, Andreas; Kippen, Marc; McBreen, Sheila; Preece, Robert; Rau, Arne; Tierney, Dave; Wilson-Hodge, Colleen

    2010-12-01

    From 2008 July to 2009 October, the Gamma-ray Burst Monitor (GBM) on board the Fermi Gamma-ray Space Telescope has detected 320 gamma-ray bursts (GRBs). About 20% of these events are classified as short based on their T 90 duration below 2 s. We present here for the first time time-resolved spectroscopy at timescales as short as 2 ms for the three brightest short GRBs observed with GBM. The time-integrated spectra of the events deviate from the Band function, indicating the existence of an additional spectral component, which can be fit by a power law with index ~-1.5. The time-integrated E peak values exceed 2 MeV for two of the bursts and are well above the values observed in the brightest long GRBs. Their E peak values and their low-energy power-law indices (α) confirm that short GRBs are harder than long ones. We find that short GRBs are very similar to long ones, but with light curves contracted in time and with harder spectra stretched toward higher energies. In our time-resolved spectroscopy analysis, we find that the E peak values range from a few tens of keV up to more than 6 MeV. In general, the hardness evolutions during the bursts follow their flux/intensity variations, similar to long bursts. However, we do not always see the E peak leading the light-curve rises and confirm the zero/short average light-curve spectral lag below 1 MeV, already established for short GRBs. We also find that the time-resolved low-energy power-law indices of the Band function mostly violate the limits imposed by the synchrotron models for both slow and fast electron cooling and may require additional emission processes to explain the data. Finally, we interpreted these observations in the context of the current existing models and emission mechanisms for the prompt emission of GRBs.

  15. The MAJORANA experiment: an ultra-low background search for neutrinoless double-beta decay

    SciTech Connect

    Phillips, D.; Aguayo Navarrete, Estanislao; Avignone, Frank T.; Back, Henning O.; Barabash, Alexander S.; Bergevin, M.; Bertrand, F.; Boswell, M.; Brudanin, V.; Busch, Matthew; Chan, Yuen-Dat; Christofferson, Cabot-Ann; Collar, J. I.; Combs, Dustin C.; Cooper, R. J.; Detwiler, Jason A.; Doe, Peter J.; Efremenko, Yuri; Egorov, Viatcheslav; Ejiri, H.; Elliott, Steven R.; Esterline, James H.; Fast, James E.; Fields, N.; Finnerty, P.; Fraenkle, Florian; Gehman, Victor; Giovanetti, G. K.; Green, Matthew P.; Guiseppe, Vincente; Gusey, K.; Hallin, A. L.; Hazama, R.; Henning, Reyco; Hime, Andrew; Hoppe, Eric W.; Horton, Mark; Howard, Stanley; Howe, M. A.; Johnson, R. A.; Keeter, K.; Keller, C.; Kidd, Mary; Knecht, A.; Kochetov, Oleg; Konovalov, S.; Kouzes, Richard T.; LaFerriere, Brian D.; LaRoque, B. H.; Leon, Jonathan D.; Leviner, L.; Loach, J. C.; MacMullin, S.; Marino, Michael G.; Martin, R. D.; Mei, Dong-Ming; Merriman, Jason H.; Miller, M. L.; Mizouni, Leila; Nomachi, Masaharu; Orrell, John L.; Overman, Nicole R.; Poon, Alan; Perumpilly, Gopakumar; Prior, Gersende; Radford, D. C.; Rielage, Keith; Robertson, R. G. H.; Ronquest, M. C.; Schubert, Alexis G.; Shima, T.; Shirchenko, M.; Snavely, Kyle J.; Steele, David; Strain, J.; Thomas, K.; Timkin, V.; Tornow, W.; Vanyushin, I.; Varner, R. L.; Vetter, Kai; Vorren, Kris R.; Wilkerson, J. F.; Wolfe, B. A.; Yakushev, E.; Young, A.; Yu, Chang-Hong; Yumatov, Vladimir; Zhang, C.

    2012-12-01

    The observation of neutrinoless double-beta decay would resolve the Majorana nature of the neutrino and could provide information on the absolute scale of the neutrino mass. The initial phase of the Majorana Experiment, known as the Demonstrator, will house 40 kg of Ge in an ultra-low background shielded environment at the 4850' level of the Sanford Underground Laboratory in Lead, SD. The objective of the Demonstrator is to validate whether a future 1-tonne experiment can achieve a background goal of one count per tonne-year in a narrow region of interest around the 76Ge neutrinoless double-beta decay peak.

  16. Simulations of electron avalanches in an ultra-low-background proportional counter

    NASA Astrophysics Data System (ADS)

    Robinson, John W.; Aalseth, Craig; Dion, Michael P.; Overman, Cory; Seifert, Allen; VanDevender, Brent

    2016-02-01

    New classes have been added to the simulation package Garfield++ to import the potential and electric field solutions generated by ANSYS ® MaxwellTM v.16. Using these tools we report results on the simulation of electron avalanches and induced signal waveforms in comparison to experimental data of the ultra-low-background gas proportional counters being developed at Pacific Northwest National Laboratory. Furthermore, an improved mesh search algorithm based on Delaunay triangulation was implemented and provided at least a three order of magnitude time savings when compared to the built-in point-location search class of Garfield++.

  17. Radioactivity of Potassium Solutions: A Comparison of Calculated Activity to Measured Activity from Gross Beta Counting and Gamma Spectroscopy

    SciTech Connect

    Gaylord, R F

    2005-07-26

    In order to determine if the measured beta activity for a solution containing potassium was exactly as predicted, particularly since the CES gas counter is not calibrated specifically with K-40, an experiment was conducted to compare measured activities from two radioanalytical methods (gamma spectroscopy and gas proportional counting) to calculated activities across a range of potassium concentrations. Potassium, being ubiquitous and naturally radioactive, is a well-known and common interference in gross beta counting methods. By measuring the observed beta activity due to K-40 in potassium-containing solutions across a wide range of concentrations, it was found that the observed beta activity agrees well with the beta activity calculated from the potassium concentration measured by standard inorganic analytical techniques, such as ICP-OES, and that using the measured potassium concentration to calculate the expected beta activity, and comparing this to the observed beta activity to determine if potassium can account for all the observed activity in a sample, is a valid technique. It was also observed that gamma spectroscopy is not an effective means of measuring K-40 activity below approximately 700 pCi/L, which corresponds to a solution with approximately 833 mg/L total potassium. Gas proportional counting for gross beta activity has a much lower detection limit, typically 20-50 picoCi/L for a liquid low in total dissolved solids, which corresponds to a potassium concentration of approximately 30-70 ppm K.

  18. Advanced performance and scalability of Si nanowire field-effect transistors analyzed using noise spectroscopy and gamma radiation techniques

    SciTech Connect

    Li, J.; Vitusevich, S. A. Pud, S.; Offenhäusser, A.; Petrychuk, M. V.; Danilchenko, B. A.

    2013-11-28

    High-quality Si nanowire field effect transistors (FETs) were fabricated using thermal nanoimprint and chemical wet etching technologies. FET structures of different lengths demonstrate high carrier mobility with values of about 750 cm{sup 2}/Vs and low volume densities of active traps in the dielectric layers of 5 × 10{sup 17} cm{sup −3} eV{sup −1}. We investigated the transport properties of these n-type channel structures using low-frequency noise spectroscopy before and after gamma radiation treatment. Before gamma irradiation, FET structures with lengths of less than 4 μm exhibited noise from contact regions with 1/(L{sup 2}) dependence for the relative 1/f noise. After gamma radiation, the spectra reflected the priority of channel noise with 1/L dependence for all samples. The transport characteristics show that the fabricated nanowire FETs improved scalability, decreased parameter scattering, and increased stability after treatment. The results demonstrate that these nanowire FETs are promising for nanoelectronic and biosensor applications due to the cost-efficient technology and advanced performance of FETs with improved stability and reliability.

  19. Spectroscopy of few-particle nuclei around magic {sup 132}Sn from fission product {gamma}-ray studies.

    SciTech Connect

    Zhang, C. T.

    1998-07-29

    We are studying the yrast structure of very neutron-rich nuclei around doubly magic {sup 132}Sn by analyzing fission product {gamma}-ray data from a {sup 248}Cm source at Eurogam II. Yrast cascades in several few-valence-particle nuclei have been identified through {gamma}{gamma} cross coincidences with their complementary fission partners. Results for two-valence-particle nuclei {sup 132}Sb, {sup 134}Te, {sup 134}Sb and {sup 134}Sn provide empirical nucleon-nucleon interactions which, combined with single-particle energies already known in the one-particle nuclei, are essential for shell-model analysis in this region. Findings for the N = 82 nuclei {sup 134}Te and {sup 135}I have now been extended to the four-proton nucleus {sup 136}Xe. Results for the two-neutron nucleus {sup 134}Sn and the N = 83 isotones {sup 134}Sb, {sup 135}Te and {sup 135}I open up the spectroscopy of nuclei in the northeast quadrant above {sup 132}Sn.

  20. The Music of the Stars : Spectroscopy of Pulsations in gamma Doradus Stars

    NASA Astrophysics Data System (ADS)

    Brunsden, Emily

    2013-05-01

    p>The mysteries of the interior structures of stars are being tackled with asteroseismology. The observable parameters of the surface pulsations of stars inform us of the interior characteristics of numerous classes of stars. The main-sequence gamma Doradus stars, just a little hotter than the Sun, offer the potential of determining stellar structure right down to the core. To determine the structural profile of a star, the observed frequencies and a full geometric description must be determined. This is only possible with long-term spectroscopic monitoring and careful analysis of the pulsation signature in spectral lines. This work seeks to identify the pulsational geometry of several gamma Doradus stars and to identify areas of improvement for current observation, analysis and modelling techniques. More than 4500 spectra were gathered on five stars for this purpose. For three stars a successful multi-frequency and mode identification solution was determined and significant progress has been made towards the understanding of a binary system involving a gamma Doradus star. A hybrid gamma Doradus/nbsp;delta Scuti pulsator was also intensely monitored and results from this work raise important questions about the classification of this type of star. Current analysis techniques were found to be fit-for-purpose for pure gamma Doradus stars, but stars with complexities such as hybrid pulsations and/or fast rotation require future development of the current models./p>

  1. Moisture logging in cased boreholes using capture gamma-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Wilson, Robert D.; Randall, Russell R.; Meisner, James E.; Boles, Jason L.; Reynolds, Kent D.

    1999-10-01

    A nuclear logging tool has been developed that determines the moisture content of subsurface earth formations by measuring the gamma rays produced by thermal neutron capture in hydrogen. The tool employs a 252Cf fast neutron source and a hyperpure germanium gamma-ray detector. The tool has demonstrated excellent sensitivity to changes in formation moisture content when used in air-filled boreholes cased with steel. The tool is also sensitive to other elements that produce neutron capture gamma rays, such as silicon, calcium, aluminum, sodium, chlorine, chromium, cadmium and mercury. Extensive computer modeling of the tool has been done to aid its design and in the interpretation of logging data taken under a variety of conditions. The logging tool has been calibrated for its moisture and chlorine response in a set of physical models and is now in use logging boreholes at the U.S. Department of Energy Hanford Site.

  2. Development of an Ultra-Low Background Liquid Scintillation Counter for Trace Level Analysis

    SciTech Connect

    Erchinger, Jennifer L.; Orrell, John L.; Aalseth, Craig E.; Bernacki, Bruce E.; Douglas, Matthew; Finn, Erin C.; Fuller, Erin S.; Keillor, Martin E.; Morley, Shannon M.; Mullen, Crystal A.; Panisko, Mark E.; Shaff, Sarah M.; Warren, Glen A.; Wright, Michael E.

    2015-09-01

    Low-level liquid scintillation counting (LSC) has been established as one of the radiation detection techniques useful in elucidating environmental processes and environmental monitoring around nuclear facilities. The Ultra-Low Background Liquid Scintillation Counter (ULB-LSC) under construction in the Shallow Underground Laboratory at Pacific Northwest National Laboratory aims to further reduce the MDAs and/or required sample processing. Through layers of passive shielding in conjunction with an active veto and 30 meters water equivalent overburden, the background reduction is expected to be 10 to 100 times below typical analytic low-background liquid scintillation systems. Simulations have shown an expected background of around 14 counts per day. A novel approach to the light collection will use a coated hollow light guide cut into the inner copper shielding. Demonstration LSC measurements will show low-energy detection, spectral deconvolution, and alpha/beta discrimination capabilities, from trials with standards of tritium, strontium-90, and actinium-227, respectively. An overview of the system design and expected demonstration measurements will emphasize the potential applications of the ULB-LSC in environmental monitoring for treaty verification, reach-back sample analysis, and facility inspections.

  3. Development of an underground low background instrument for high sensitivity measurements

    NASA Astrophysics Data System (ADS)

    Sala, E.; Hahn, I. S.; Kang, W. G.; Kim, G. W.; Kim, Y. D.; Lee, M. H.; Leonard, D. S.; Park, Su Yeon

    2016-05-01

    The Center for Underground Physics has developed in collaboration with CANBERRA a low background instrument composed of 14 HPGe detectors divided in two arrays facing each other. The performance and the background of a single detector of the array have been studied in order to improve the array final configuration. An accurate material selection, through the measurements of building material samples and Monte Carlo simulations based on Geant4, has been performed to reach the lowest possible intrinsic background. Alternative materials and configurations have been considered for the final design of the array simulating the expected intrinsic background of the instrument considering the needed changes. The expected sensitivity of the improved array configuration, concerning the low background material selection for rare events physics experiments, has been evaluated through Monte Carlo simulations considering 232Th concentration in a Copper sample. Since the array can also be used for rare decays searches, the expected sensitivity on the 156Dy resonant double electron capture has thus been calculated.

  4. Non-destructive determination of 224Ra, 226Ra and 228Ra concentrations in drinking water by gamma spectroscopy.

    PubMed

    Parekh, Pravin; Haines, Douglas; Bari, Abdul; Torres, Miguel

    2003-11-01

    The U.S. Environmental Protection Agency mandates that drinking water showing gross alpha-activity greater than 0.19 Bq L(-1) should be analyzed for radium, a known human carcinogen. The recommended testing methods are intricate and laborious. The method reported in this paper is a direct, non-destructive gamma-spectroscopic method for the determination of 224Ra, 226Ra, and 228Ra, the three radium isotopes of environmental concern in drinking water. Large-volume Marinelli beakers (4.1-L capacity), especially designed for measuring radioactive gases, in conjunction with a low-background, high-efficiency (131%) germanium detector were used in this work. It was first established that radon, the gaseous decay product of radium, and its progeny are quantitatively retained in this Marinelli beaker. The 224Ra, 226Ra, and 228Ra activity concentrations are determined from the equilibrium activities of their progeny: 212Pb, 214Pb (214Bi), and 228Ac; and the gamma-lines used in the analysis are 238.6, 351.9 (and 609.2), and 911.2 keV, respectively. The 224Ra activity is determined from the first 1,000-min measurement performed after expulsion of radon from the sample. The 226Ra activity is determined from the second, 2,400-min measurement, made 3 to 5 d later, and the 228Ra activity is determined from either the first or the second measurement, depending on its concentration level. The method's minimum detectable activities are 0.017 Bq L(-1), 0.020 Bq L(-1), and 0.027 Bq L(-1) for 224Ra, 226Ra, and 228Ra, respectively, when measured under radioactive equilibrium. These limits are well within the National Primary Drinking Water Regulations required limit of 0.037 Bq L(-1) for 226Ra and for 228Ra. The precision and accuracy of the method, evaluated using the U.S. Environmental Protection Agency and the Environmental Resource Associates' quality control samples, were found to be within acceptable limits. PMID:14571995

  5. Development of a detector based on Silicon Drift Detectors for gamma-ray spectroscopy and imaging applications

    NASA Astrophysics Data System (ADS)

    Busca, P.; Butt, A. D.; Fiorini, C.; Marone, A.; Occhipinti, M.; Peloso, R.; Quaglia, R.; Bombelli, L.; Giacomini, G.; Piemonte, C.; Camera, F.; Giaz, A.; Million, B.; Nelms, N.; Shortt, B.

    2014-05-01

    This work deals with the development of a new gamma detector based on Silicon Drift Detectors (SDDs) to readout large LaBr3:Ce scintillators for gamma-ray spectroscopy and imaging applications. The research is supported by the European Space Agency through the Technology Research Programme (TRP) and by Istituto Nazionale di Fisica Nucleare (INFN) within the Gamma project. The SDDs, produced at Fondazione Bruno Kessler (FBK) semiconductor laboratories, are designed as monolithic arrays of 3 × 3 units, each one of an active area of 8 mm × 8 mm (overall area of 26 mm × 26 mm). The readout electronics and the architecture of the camera are briefly described and then first experimental results coupling the SDD array with a 1'' × 1'' LaBr3:Ce scintillator are reported. An energy resolution of 3% FWHM at 662 keV has been measured at -20°C, better than coupling the same scintillator with a photomultiplier tube. The same scintillator is also used to evaluate position sensitivity with a 1 mm collimated Cs-137 source. The main difficulty in determining the position of the gamma-ray interaction in the crystal is associated to the high thickness/diameter ratio of the crystal (1:1) and the use of reflectors on all lateral and top sides the crystal. This last choice enhances energy resolution but makes imaging capability more challenging because light is spread over all photodetectors. Preliminary results show that the camera is able to detect shifts in the measured signals, when the source is moved with steps of 5 mm. A modified version of the centroid method is finally implemented to evaluate the imaging capability of the system.

  6. Metabolic Study of Breast MCF-7 Tumor Spheroids after Gamma Irradiation by 1H NMR Spectroscopy and Microimaging

    PubMed Central

    Palma, Alessandra; Grande, Sveva; Luciani, Anna Maria; Mlynárik, Vladimír; Guidoni, Laura; Viti, Vincenza; Rosi, Antonella

    2016-01-01

    Multicellular tumor spheroids are an important model system to investigate the response of tumor cells to radio- and chemotherapy. They share more properties with the original tumor than cells cultured as 2D monolayers do, which helps distinguish the intrinsic properties of monolayer cells from those induced during cell aggregation in 3D spheroids. The paper investigates some metabolic aspects of small tumor spheroids of breast cancer and their originating MCF-7 cells, grown as monolayer, by means of high–resolution (HR) 1H NMR spectroscopy and MR microimaging before and after gamma irradiation. The spectra of spheroids were characterized by higher intensity of mobile lipids, mostly neutral lipids, and glutamine (Gln) signals with respect to their monolayer cells counterpart, mainly owing to the lower oxygen supply in spheroids. Morphological changes of small spheroids after gamma-ray irradiation, such as loss of their regular shape, were observed by MR microimaging. Lipid signal intensity increased after irradiation, as evidenced in both MR localized spectra of the single spheroid and in HR NMR spectra of spheroid suspensions. Furthermore, the intense Gln signal from spectra of irradiated spheroids remained unchanged, while the low Gln signal observed in monolayer cells increased after irradiation. Similar results were observed in cells grown in hypoxic conditions. The different behavior of Gln in 2D monolayers and in 3D spheroids supports the hypothesis that a lower oxygen supply induces both an upregulation of Gln synthetase and a downregulation of glutaminases with the consequent increase in Gln content, as already observed under hypoxic conditions. The data herein indicate that 1H NMR spectroscopy can be a useful tool for monitoring cell response to different constraints. The use of spheroid suspensions seems to be a feasible alternative to localized spectroscopy since similar effects were found after radiation treatment. PMID:27200293

  7. Continuous versus pulse neutron induced gamma spectroscopy for soil carbon analysis

    Technology Transfer Automated Retrieval System (TEKTRAN)

    Neutron induced gamma spectra analysis (NGA) provides a means of measuring carbon in large soil volumes without destructive sampling. Calibration of the NGA system must account for system background and the interference of other nuclei on the carbon peak at 4.43 MeV. Accounting for these factors pro...

  8. Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

    SciTech Connect

    Ludewigt, Bernhard; Mozin, Vladimir; Campbell, Luke; Favalli, Andrea; Hunt, Alan W.; Reedy, Edward T.E.; Seipel, Heather A.

    2015-09-28

    This project has been a collaborative effort of researchers from four National Laboratories, Lawrence Berkley National Laboratory (LBNL), Lawrence Livermore National Laboratory (LLNL), Los Alamos National Laboratory (LANL), Pacific Northwest National Laboratory (PNNL), and Idaho State University’s (ISU) Idaho Accelerator Center (IAC). Experimental measurements at the Oregon State University (OSU) were also supported. The research included two key components, a strong experimental campaign to characterize the delayed gamma-ray signatures of the isotopes of interests and of combined targets, and a closely linked modeling effort to assess system designs and applications. Experimental measurements were performed to evaluate fission fragment yields, to test methods for determining isotopic fractions, and to benchmark the modeling code package. Detailed signature knowledge is essential for analyzing the capabilities of the delayed gamma technique, optimizing measurement parameters, and specifying neutron source and gamma-ray detection system requirements. The research was divided into three tasks: experimental measurements, characterization of fission yields, and development of analysis methods (task 1), modeling in support of experiment design and analysis and for the assessment of applications (task 2), and high-rate gamma-ray detector studies (task 3).

  9. {gamma}-ray spectroscopy of the neutron-rich nuclei {sup 89}Rb, {sup 92}Y, and {sup 93}Y with multinucleon transfer reactions

    SciTech Connect

    Bucurescu, D.; Ionescu-Bujor, M.; Iordachescu, A.; Mihai, C.; Suliman, G.; Rusu, C.; Marginean, N.; Ur, C. A.; Marginean, R.; De Angelis, G.; Corradi, L.; Vedova, F. Della; Fioretto, E.; Gadea, A.; Guiot, B.; Napoli, D.; Stefanini, A. M.; Valiente-Dobon, J. J.; Bazzacco, D.; Beghini, S.

    2007-12-15

    The positive-parity yrast states in the {sup 89}Rb, {sup 92}Y, and {sup 93}Y nuclei were studied using {gamma}-ray spectroscopy with heavy-ion induced reactions. In the multinucleon transfer reactions {sup 208}Pb+{sup 90}Zr (590 MeV) and {sup 238}U+{sup 82}Se (505 MeV), several {gamma}-ray transitions were identified in these nuclei by means of coincidences between recoiling ions identified with the PRISMA spectrometer and {gamma} rays detected with the CLARA {gamma}-ray array in thin target experiments. Level schemes were subsequently determined from triple-{gamma} coincidences recorded with the GASP array in a thick target experiment, in the reactions produced by a 470 MeV {sup 82}Se beam with a {sup 192}Os target. The observed level schemes are compared to shell-model calculations.

  10. Low-background performance of a monolithic InSb CCD array

    NASA Technical Reports Server (NTRS)

    Bregman, J. D.; Goebel, J. H.; Mccreight, C. R.; Matsumoto, T.

    1982-01-01

    A 20 element monolithic InSb charge coupled device (CCD) detector array was measured under low background conditions to assess its potential for orbital astronomical applications. At a temperature of 64 K, previous results for charge transfer efficiency (CTE) were reproduced, and a sensitivity of about 2 x 10 to the minus 15th power joules was measured. At 27 and 6 K, extended integration times were achieved, but CTE was substantially degraded. The noise was approximately 6000 charges, which was in excess of the level where statistical fluctuations from the illumination could be detected. A telescope demonstration was performed showing that the array sensitivity and difficulty of operation were not substantially different from laboratory levels. Ways in which the device could be improved for astronomical applications were discussed.

  11. Estimation of Equivalent Sea Level Cosmic Ray Exposure for Low Background Experiment

    SciTech Connect

    Greene, Austen T.; Orrell, John L.

    2012-08-25

    While scientists at CERN and other particle accelerators around the world explore the boundaries of high energy physics, the Majorana project investigates the other end of the spectrum with its extremely sensitive, low background, low energy detector. The MAJORANA DEMONSTRATOR aims to detect neutrinoless double beta decay (0νββ), a rare theoretical process in which two neutrons decay into two protons and two electrons, without the emission of the two antineutrinos that are a product of a normal double beta decay. This process is only possible if – and therefore a detection would prove — the neutrino is a Majorana particle, meaning that it is its own antiparticle [Aaselth et al. 2004] . The existence of such a decay would also disprove lepton conservation and give information about the neutrino's mass.

  12. Studies with a low-background germanium detector in the Holborn Underground laboratory

    NASA Astrophysics Data System (ADS)

    Barton, J. C.

    1995-02-01

    This paper reports on the performance and use of a low background HPGe detector, which was operated in the Holborn Underground laboratory from May 1990 to July 1993, and on some of the results obtained from it. The analysis includes sections on measuring the efficiency of the system and a discussion of the contributions to the background. Most of the materials studied were those being considered for use in the Solar Neutrino Observatory or in the UK Dark Matter programme. Results for the natural radioactivity in various classes of materials include those for the glass used in photomultipliers, the extent of non-equilibrium in the main decay series of thorium and uranium and the presence of protactinium in samples of zirconium oxide. There is also a summary of the cosmogenic isotopes found in the meteorite Glatton which fell in 1991.

  13. InSb 288*32 FPA with digital TDI for low background application

    NASA Astrophysics Data System (ADS)

    Chishko, V. F.; Kasatkin, I. L.; Lopukhin, A. A.

    2007-05-01

    32*288 format FPA based on InSb two dimension arrays (IDA) of photodiodes with function of digital TDI were investigated at low background flow. Dark currents of TDA photodiodes in wide temperature region, spectral noise distribution and threshold power with TDI simulation are investigated. It was established that at T=77K dark current is (I - 3)*10-11A at optimal negative bias and decreases in the order of magnitude at T=65K. Threshold power at T=77K at integration time Ti=6 ms is not more 2*10 -14 W/pixel and is limited commonly by dark current noise. Modeling of digital TDI showed that not more than twenty TDI stages are effective because of the presence of 1/f noise and threshold power would be at about 3*10 -15 W/pixel.

  14. Low-background measurements of neutron emission from Ti metal in pressurized deuterium gas

    SciTech Connect

    Menlove, H.O.; Paciotti, M.A.; Claytor, T.N.; Tuggle, D.G.

    1991-01-01

    A wide variety of neutron detector systems have been used at various research facilities to search for anomalous neutron emission from deuterated metals. Some of these detector systems are summarized here together with possible sources of spurious signals from electronic noise. During the past two years, we have performed experiments to measure neutron emission from pressurized D{sub 2} gas mixed with various forms of titanium metal chips and sponge. Details concerning the neutron detectors, experimental procedures, and results have been reported previously. Our recent experiments have focused on increasing the low-level neutron emission and finding a way to trigger the emission. To improve our detection sensitivity, we have increased the shielding in our counting laboratory, changed to low-background {sup 3}He tubes, and set up additional detector systems in deep underground counting stations. This report is an update on this experimental work. 7 refs., 5 figs., 4 tabs.

  15. Investigations of 2β decay measured by low background HPGe spectrometer OBELIX

    SciTech Connect

    Rukhadze, Ekaterina [Institute of Experimental and Applied Physics, CTU in Prague, Horska 3a Collaboration: OBELIX Collaboration; SuperNEMO Collaboration

    2013-12-30

    A low background high sensitive HPGe spectrometer OBELIX was installed at the Modane Underground Laboratory (LSM, France, 4800 m w.e.). The detector was designed to measure a contamination of enriched isotopes and radio-impurities in construction materials, to investigate rare nuclear processes such as resonance neutrinoless double electron capture and two-neutrino double beta decay to excited states of daughter nuclei. Spectrometer sensitivity, contamination of NEMO-3 sources and results of 2ν2β{sup −} decay of {sup 100}Mo to the 0{sup +} (1130 keV) and 2{sup +} (540 keV) excited states as well as future plans for OBELIX detector are given.

  16. The Design of an Ultra-Low Background Thermosyphon for the Majorana Demonstrator

    SciTech Connect

    Aguayo Navarrete, Estanislao; Busch, Matthew; Daniels, Randy; Fast, James E.; Green, Matthew P.; Reid, Douglas J.

    2013-05-01

    The MAJORANA DEMONSTRATOR (MJD) is an ultra-low background neutrinoless double-beta decay (0νββ) experiment that will deploy up to 40 kg of high purity germanium detectors (HPGe). The goal of this experiment is to demonstrate the feasibility of building a detector array with less than 1 event/ton-year in a 4 keV region of interest around the 0νββ signal. HPGe diodes, when used as ionizing radiation detectors, need to be maintained at a temperature close to that of liquid nitrogen (77 K). This work describes the R&D results of a cryogenic system capable of meeting the requirements of low background and the cooling capacity required to successfully operate such a detector system. The MJD germanium detector modules will operate at liquid nitrogen temperature to provide adequate cooling for a full range of HPGe impurity concentrations. This paper shows the experimental results obtained using a two-phase horizontal thermosyphon using liquid nitrogen as the MJD’s cooling system. The cold test shows that the proposed thermosyphon has sufficient cooling power to handle the heat load of an MJD module. Results for the temperature gradient across the thermosyphon, cooling capacity, and design considerations demonstrate that the thermosyphon can effectively remove the calculated heat load of each module of the experiment. The thermosyphon will be bolted to a cold plate from which detector strings will hang. The thermal conductivity of a mockup of the MJD bolted thermal joint is experimentally determined to be below 0.1 K/W.

  17. High resolution gamma-ray spectroscopy applied to bulk sample analysis

    SciTech Connect

    Kosanke, K.L.; Koch, C.D.; Wilson, R.D.

    1980-01-01

    A high resolution Ge(Li) gamma-ray spectrometer has been installed and made operational for use in routine bulk sample analysis by the Bendix Field Engineering Corporation (BFEC) geochemical analysis department. The Ge(Li) spectrometer provides bulk sample analyses for potassium, uranium, and thorium that are superior to those obtained by the BFEC sodium iodide spectrometer. The near term analysis scheme permits a direct assay for uranium that corrects for bulk sample self-absorption effects and is independent of the uranium/radium disequilibrium condition of the sample. A more complete analysis scheme has been developed that fully utilizes the gamma-ray data provided by the Ge(Li) spectrometer and that more properly accounts for the sample self-absorption effect. This new analysis scheme should be implemented on the BFEC Ge(Li) spectrometer at the earliest date.

  18. Investigation of Martian H2O and CO2 via gamma-ray spectroscopy

    NASA Technical Reports Server (NTRS)

    Squyres, Steven W.; Evans, Larry G.

    1987-01-01

    The evolution and present state of water and carbon dioxide on Mars are discussed. Researchers wished to determine how effectively questions regarding the distribution of water and carbon dioxide on Mars may be addressed with orbital gamma ray spectrometer data. Several simple, multi-layer models of the Martian surface were formulated to address problems such as the ice/dust ratio of layered deposits; the distribution, depth and concentration of ground ice; the thickness of north polar perennial ice; the thickness of the carbon dioxide layer over the south polar cap; the thickness of the seasonal carbon dioxide frost cap; and the water content of the seasonal frost cap. The results indicate that the Mars Observer gamma ray spectrometer will be a powerful tool for investigating the distribution and stratigraphy of volatiles on Mars.

  19. Topics in Astrophysical X-Ray and Gamma Ray Spectroscopy. Ph.D. Thesis - Maryland Univ.

    NASA Technical Reports Server (NTRS)

    Bussard, R. W.

    1978-01-01

    A number of topics relating to astrophysical observations that have already been made or are currently planned of spectral features, mostly emission lines, in the X-ray and gamma ray region of the electromagnetic spectrum are investigated. These topics include: the production of characteristic X-ray and gamma ray lines by nonthermal ions, spectral features induced by processes occurring in strong magnetic fields, and the positron annihilation line at 0.5 MeV. The rate of X-ray production at 6.8 keV by the 2p to 1s transition in fast hydrogen- and helium-like iron ions, following both electron capture to excited levels and collisional excitation is calculated. The cross section for electron-ion Coulomb collisions in strong fields is also calculated.

  20. GAMIDEN: a program to aid in the identification of unknown materials by gamma-ray spectroscopy

    SciTech Connect

    Howerton, R.J.

    1983-05-10

    The intent of the computer code GAMIDEN is to help identify isotopes by their gamma-ray emissions and thus to assist in the nondestructive assay of unknown materials. From both radioactive decays and neutron captures, GAMIDEN searches GAMTOT83, a file of gamma-ray spectra, for matches with observed photon energies. This report describes the search procedure, outlines the use of the code, and gives an example. The code is designed to operate on the CRAY 1 computer at Lawrence Livermore National Laboratory (LLNL). It is written in standard Fortran (ANSI) for the most part but contains some LRLTRAN instructions to make use of the Livermore time-sharing system (LTSS). The code uses about 545,000 words of memory. Typical problems run in about 45 s. The source program and the data file are available on request.

  1. High resolution X- and gamma-ray spectroscopy of cosmic X-ray sources

    NASA Technical Reports Server (NTRS)

    Lin, R. P.

    1983-01-01

    A high resolution X-ray spectrometer and large area phoswich detector were designed and co-aligned in a common elevation mounting in order to measure solar and cosmic X-ray and gamma ray emission in the 13 to 600 KeV energy range from a balloon. The instrument is described and results obtained for the Crab Nebula, the supernova remnant Cas A, and the Sun are discussed and analyzed.

  2. Spectroscopy of the B-gamma line in the Galactic center

    NASA Technical Reports Server (NTRS)

    Nadeau, D.; Neugebauer, G.; Matthews, K.; Geballe, T. R.

    1981-01-01

    Spectra of the B-gamma recombination line of hydrogen in the Galactic center show that the line has central velocities and shapes similar to those reported previously for the Ne II line. Observations are made at 10 positions within the infrared cluster of the Galactic center with a circular diaphragm of diameter 5 arcsec and with a spectral resolution of approximately 85 km/sec. The spectra confirm that the ionized gas in the Galactic center is distributed in discrete clouds.

  3. Total absorption {gamma}-ray spectroscopy of beta delayed neutron emitters

    SciTech Connect

    Valencia, E.; Algora, A.; Tain, J. L.; Agramunt, J.; Jordan, M. D.; Molina, F.; Estevez, E.; Rubio, B.; Perez, A.; Rice, S.; Bowry, M.; Gelletly, W.; Podolyak, Zs.; Regan, P. H.; Farrelly, G. F.; Zakari-Issoufou, A.-A.; Porta, A.; Fallot, M.; Bui, V. M.; and others

    2013-06-10

    Preliminary results of the data analysis of the beta decay of {sup 94}Rb using a novel - segmented- total absorption spectrometer are shown in this contribution. This result is part of a systematic study of important contributors to the decay heat problem in nuclear reactors. In this particular case the goal is to determine the beta intensity distribution below the neutron separation energy and the gamma/beta competition above.

  4. Spectroscopy of {sup 189,187}Pb from gamma-FMA coincidences

    SciTech Connect

    Janssens, R.V.F.; Davids, C.N.; Blumenthal, D.

    1995-08-01

    The very neutron-deficient Pb isotopes are of much current interest because they exhibit shape coexistence between a spherical groundstate and a deformed prolate excited configuration located very low in excitation energy. Last year the nucleus {sup 186}Pb was studied at the FMA in an FMA-{gamma}-{gamma} coincidence experiment. The purpose of the present measurement was to delineate, for the first time, the groundstate and near groundstate excitations in the odd Pb isotopes {sup 189,187}Pb in order to identify the orbitals which have an important role in driving the nuclear shape. The experiment was performed only very recently at the FMA with 10 Compton-suppressed Ge detectors from the Argonne Notre Dame BGO Gamma-Ray facility. {sup 187}Pb was studied with the {sup 155}Gd({sup 36}Ar,4n) reaction at 179 MeV, while {sup 189}Pb was reached with the {sup 158}Gd({sup 36}Ar,5n) reaction at the same beam energy. The analysis just began. It can already be stated that transitions in both Pb isotopes were identified and that it should be possible to establish level schemes. The presence of possible isomeric states in {sup 189}Pb will be checked in a follow-up experiment planned in Canberra. A similar measurement on {sup 187}Pb appears very difficult because of the very small cross section involved.

  5. Coupling Deterministic and Monte Carlo Transport Methods for the Simulation of Gamma-Ray Spectroscopy Scenarios

    SciTech Connect

    Smith, Leon E.; Gesh, Christopher J.; Pagh, Richard T.; Miller, Erin A.; Shaver, Mark W.; Ashbaker, Eric D.; Batdorf, Michael T.; Ellis, J. E.; Kaye, William R.; McConn, Ronald J.; Meriwether, George H.; Ressler, Jennifer J.; Valsan, Andrei B.; Wareing, Todd A.

    2008-10-31

    Radiation transport modeling methods used in the radiation detection community fall into one of two broad categories: stochastic (Monte Carlo) and deterministic. Monte Carlo methods are typically the tool of choice for simulating gamma-ray spectrometers operating in homeland and national security settings (e.g. portal monitoring of vehicles or isotope identification using handheld devices), but deterministic codes that discretize the linear Boltzmann transport equation in space, angle, and energy offer potential advantages in computational efficiency for many complex radiation detection problems. This paper describes the development of a scenario simulation framework based on deterministic algorithms. Key challenges include: formulating methods to automatically define an energy group structure that can support modeling of gamma-ray spectrometers ranging from low to high resolution; combining deterministic transport algorithms (e.g. ray-tracing and discrete ordinates) to mitigate ray effects for a wide range of problem types; and developing efficient and accurate methods to calculate gamma-ray spectrometer response functions from the deterministic angular flux solutions. The software framework aimed at addressing these challenges is described and results from test problems that compare coupled deterministic-Monte Carlo methods and purely Monte Carlo approaches are provided.

  6. High resolution X- and gamma-ray spectroscopy of solar flares

    NASA Technical Reports Server (NTRS)

    Lin, R. P.

    1984-01-01

    A balloon-borne X- and gamma-ray instrument was developed, fabricated, and flown. This instrument has the highest energy resolution of any instrument flown to date for measurements of solar and cosmic X-ray and gamma-ray emission in the 13 to 600 keV energy range. The purpose of the solar measurements was to study electron acceleration and solar flare energy release processes. The cosmic observations were to search for cyclotron line features from neutron stars and for low energy gamma-ray lines from nucleosynthesis. The instrument consists of four 4 cm diameter, 1.3 cm thick, planar intrinsic germanium detectors cooled by liquid nitrogen and surrounded by CsI and NaI anti-coincidence scintillation crystals. A graded z collimator limited the field of view to 3 deg x 6 deg and a gondola pointing system provided 0.3 deg pointing accuracy. A total of four flights were made with this instrument. Additional funding was obtained from NSF for the last three flights, which had primarily solar objectives. A detailed instrument description is given. The main scientific results and the data analysis are discussed. Current work and indications for future work are summarized. A bibliography of publications resulting from this work is given.

  7. Study of the Nuclear Structure of 39P Using Beta-Delayed Gamma Spectroscopy

    NASA Astrophysics Data System (ADS)

    Abromeit, Brittany; NSCL Experiment E14063 Team Team

    2016-03-01

    Investigation of nuclei with neutron and proton imbalance is at the forefront of nuclear physics research today. This is driven by the fact that the structure in these regimes may vary with that seen near the valley of stability. With eight neutrons more than the stable isotope of phosphorous, 39P is a neutron-rich exotic nucleus that has very limited information on it: previous studies of 39P produce only three known energy levels and gamma rays. The fragmentation of a 48Ca primary beam on a 564mg/cm2 thick Be target at the National Superconducting Cyclotron Laboratory (NSCL) was used to produce exotic 39Si. Using the NSCL Beta Counting System (BCS), consisting of a thick planner germanium double-sided strip detector (GeDSSD) and 16 High-purity germanium detectors in an array, SeGA, the beta-gamma coincidences from the decay of 39Si to 39P were analyzed. The resulting level scheme of 39P, including over 12 new gamma rays and energy states, confirmation of the previously measured half-life, and first-time logft values will be presented. This work was supported by the NSF under Grant No. 1401574.

  8. Feasibility study of in vivo partial body potassium determination in the human body using gamma-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Ramirez, Lisa Marie

    This work investigates partial body potassium determination in the human body using gamma-ray spectroscopy. Potassium is an essential element in the human body that controls many of the enzyme systems and intra- and extra-cellular water flow. Potassium is symptomatic to several disease cases and has gender and ethnic variability. This work assesses the feasibility to measure partial body potassium in three specific regions: brain, arm, and leg, that are of interest to multiple sclerosis, chronic renal failure, and spinal cord injury, respectively. Three detector systems were constructed and their capabilities assessed. System characterization and analytical procedure for potassium evaluation and determination are presented together with experimental and initial clinical results. The results indicate that partial body potassium measurement is viable, statistically reproducible, and has potential clinical significance.

  9. OPTIMIZATION OF VIRTUAL FRISCH-GRID CdZnTe DETECTOR DESIGNS FOR IMAGING AND SPECTROSCOPY OF GAMMA RAYS.

    SciTech Connect

    BOLOTNIKOV,A.E.; ABDUL-JABBAR, N.M.; BABALOLA, S.; CAMARDA, G.S.; CUI, Y.; HOSSAIN, A.; JACKSON, E.; JACKSON, H.; JAMES, J.R.; LURYI, A.L.; JAMES, R.B.

    2007-08-21

    In the past, various virtual Frisch-grid designs have been proposed for cadmium zinc telluride (CZT) and other compound semiconductor detectors. These include three-terminal, semi-spherical, CAPture, Frisch-ring, capacitive Frisch-grid and pixel devices (along with their modifications). Among them, the Frisch-grid design employing a non-contacting ring extended over the entire side surfaces of parallelepiped-shaped CZT crystals is the most promising. The defect-free parallelepiped-shaped crystals with typical dimensions of 5x5{approx}12 mm3 are easy to produce and can be arranged into large arrays used for imaging and gamma-ray spectroscopy. In this paper, we report on further advances of the virtual Frisch-grid detector design for the parallelepiped-shaped CZT crystals. Both the experimental testing and modeling results are described.

  10. Photon Activation Analysis Of Light Elements Using 'Non-Gamma' Radiation Spectroscopy - The Instrumental Determination Of Phosphorus

    SciTech Connect

    Segebade, Christian; Goerner, Wolf

    2011-06-01

    Unlike metal determinations the analysis of light elements (e.g., carbon, oxygen, phosphorus) is frequently problematic, in particular if analysed instrumentally. In photon activation analysis (PAA) the respective activation products do not emit gamma radiation in the most cases. Usually, annihilation quanta counting and subsequent decay curve analysis have been used for determinations of C, N, O, and F. However, radiochemical separation of the respective radioisotopes mostly is indispensable. For several reasons, some of the light elements cannot be analysed following this procedure, e.g. phosphorus. In this contribution the instrumental PAA of phosphorus in organic matrix by activation with bremsstrahlung of an electron linear accelerator and subsequent beta spectroscopy is described. The accuracy of the results was excellent as obtained by analysis of a BCR Reference Material.

  11. High-resolution gamma-ray spectroscopy with a microwave-multiplexed transition-edge sensor array

    SciTech Connect

    Noroozian, Omid; Mates, John A. B.; Bennett, Douglas A.; Brevik, Justus A.; Fowler, Joseph W.; Gao, Jiansong; Hilton, Gene C.; Horansky, Robert D.; Irwin, Kent D.; Schmidt, Daniel R.; Vale, Leila R.; Ullom, Joel N.; Kang, Zhao

    2013-11-11

    We demonstrate very high resolution photon spectroscopy with a microwave-multiplexed two-pixel transition-edge sensor (TES) array. We measured a {sup 153}Gd photon source and achieved an energy resolution of 63 eV full-width-at-half-maximum at 97 keV and an equivalent readout system noise of 86 pA/√(Hz) at the TES. The readout circuit consists of superconducting microwave resonators coupled to radio-frequency superconducting-quantum-interference-devices and transduces changes in input current to changes in phase of a microwave signal. We use flux-ramp modulation to linearize the response and evade low-frequency noise. This demonstration establishes one path for the readout of cryogenic X-ray and gamma-ray sensor arrays with more than 10{sup 3} elements and spectral resolving powers R=λ/Δλ>10{sup 3}.

  12. Radiological Assessment of Natural and Artificial Radionuclides in Mission (Texas) Surface Soils via Gamma-ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Wahid, Kareem; Hannan, Mohammad; Nguyen, Nam

    2015-04-01

    Residents living near decommissioned chemical facilities in the city of Mission, Texas have been noted to complain of physiological abnormalities and health related problems associated with low dose radiation exposure. The purpose of this study was to quantify radioactivity levels in the entire Mission area by measuring natural and anthropogenic radionuclide concentrations in 30 representative surface soil samples through high-resolution gamma-ray spectroscopy. The mean specific activity concentrations for these radionuclides were similar to other comparable locations and followed an approximately normal distribution across the samples. In addition, radiological impact assessment factors such as the absorbed dose rate, annual effective dose, radium equivalent activity, and external radiation hazard index were calculated and found to be lower than recommended values, thereby signifying that there seems to be no potential radiological threat associated with Mission surface soils.

  13. OSIRIS-Gamma-ray spectroscopy software for on-site inspections under the Comprehensive Nuclear-Test-Ban Treaty

    NASA Astrophysics Data System (ADS)

    Caffrey, A. J.; Bowyer, T. W.; Egger, A. E.; Hall, J. C.; Kelly, S. M.; Krebs, K. M.; Kreek, S. A.; Jordan, D. V.; Milbrath, B. D.; Padgett, S. W.; Wharton, C. J.; Wimer, N. G.

    2015-06-01

    We have designed and tested software for the acquisition and analysis of high-resolution gamma-ray spectra during on-site inspections under the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The On-Site Inspection RadioIsotopic Spectroscopy-OSIRIS-software filters the spectral data to display only radioisotopic information relevant to CTBT on-site inspections, e.g.,131I. A set of over 100 fission-product spectra was employed for OSIRIS testing. These spectra were measured where possible, or generated by modeling. The test spectral compositions include non-nuclear-explosion scenarios, e.g., a severe nuclear reactor accident, and nuclear-explosion scenarios such as a vented underground nuclear test. Comparing its computer-based analyses to expert visual analyses of the test spectra, OSIRIS correctly identifies CTBT-relevant fission product isotopes at the 95% level or better.

  14. Optimization of virtual Frisch-grid CdZnTe detector designs for imaging and spectroscopy of gamma rays

    NASA Astrophysics Data System (ADS)

    Bolotnikov, A. E.; Abdul-Jabbar, N. M.; Babalola, S.; Camarda, G. S.; Cui, Y.; Hossain, A.; Jackson, E.; Jackson, H.; James, J. R.; Luryi, A. L.; James, R. B.

    2007-09-01

    In the past, various virtual Frisch-grid designs have been proposed for cadmium zinc telluride (CZT) and other compound semiconductor detectors. These include three-terminal, semi-spherical, CAPture, Frisch-ring, capacitive Frisch-grid and pixel devices (along with their modifications). Among them, the Frisch-grid design employing a non-contacting ring extended over the entire side surfaces of parallelepiped-shaped CZT crystals is the most promising. The defect-free parallelepiped-shaped crystals with typical dimensions of 5x5x12 mm3 are easy to produce and can be arranged into large arrays used for imaging and gamma-ray spectroscopy. In this paper, we report on further advances of the virtual Frisch-grid detector design for the parallelepiped-shaped CZT crystals. Both the experimental testing and modelling results are described.

  15. Laboratory Studies of Lead Removal from Liquid Scintillator in Preparation for KamLAND's Low Background Phase

    SciTech Connect

    Keefer, Gregory

    2011-04-27

    The removal of Radon induced Lead from liquid scintillator was extensively studied in preparation for KamLAND's low background phase. This work presents the results from laboratory experiments performed at the University of Alabama and their implications for KamLAND and future low background experiments using carbon based liquid scintillator. It was observed that distillation was the most effective purification procedure and that one must consider a non-polar and non-ionic component of Lead in order to reach the levels of radio-purity required for these new class of ultra-low background experiments.

  16. Dual sightline measurements of MeV range deuterons with neutron and gamma-ray spectroscopy at JET

    NASA Astrophysics Data System (ADS)

    Eriksson, J.; Nocente, M.; Binda, F.; Cazzaniga, C.; Conroy, S.; Ericsson, G.; Giacomelli, L.; Gorini, G.; Hellesen, C.; Hellsten, T.; Hjalmarsson, A.; Jacobsen, A. S.; Johnson, T.; Kiptily, V.; Koskela, T.; Mantsinen, M.; Salewski, M.; Schneider, M.; Sharapov, S.; Skiba, M.; Tardocchi, M.; Weiszflog, M.; Contributors, JET

    2015-11-01

    Observations made in a JET experiment aimed at accelerating deuterons to the MeV range by third harmonic radio-frequency (RF) heating coupled into a deuterium beam are reported. Measurements are based on a set of advanced neutron and gamma-ray spectrometers that, for the first time, observe the plasma simultaneously along vertical and oblique lines of sight. Parameters of the fast ion energy distribution, such as the high energy cut-off of the deuteron distribution function and the RF coupling constant, are determined from data within a uniform analysis framework for neutron and gamma-ray spectroscopy based on a one-dimensional model and by a consistency check among the individual measurement techniques. A systematic difference is seen between the two lines of sight and is interpreted to originate from the sensitivity of the oblique detectors to the pitch-angle structure of the distribution around the resonance, which is not correctly portrayed within the adopted one dimensional model. A framework to calculate neutron and gamma-ray emission from a spatially resolved, two-dimensional deuteron distribution specified by energy/pitch is thus developed and used for a first comparison with predictions from ab initio models of RF heating at multiple harmonics. The results presented in this paper are of relevance for the development of advanced diagnostic techniques for MeV range ions in high performance fusion plasmas, with applications to the experimental validation of RF heating codes and, more generally, to studies of the energy distribution of ions in the MeV range in high performance deuterium and deuterium-tritium plasmas.

  17. Method and apparatus for determining the respective contributions of borehole and earth formation in gamma ray spectroscopy

    SciTech Connect

    Stoller, C.; Adolph, R.A.

    1992-04-14

    This patent describes a method for determining the respective contributions in spectroscopy measurements of the borehole and the earth formations surrounding the borehole. It comprises: irradiating the formation with neutrons from a high energy neutron source; detecting and counting, at each depth in the borehole, at least a first and a second location, the gamma rays resulting from the interaction of the neutrons with atoms of the formation and the borehole; forming, for each depth, a first and a second gamma ray response for respectively the first and second detection location, the responses being representative of at least an unknown parameter of the formation and/or the borehole; cross-plotting each of the first responses versus the corresponding second response; thus, with each depth is associated on the cross-plot a dot representing the set of first-/second responses for that depth; deriving from known conditions of the detection, and from the general relationship between the responses and the unknown parameter, a closed curve characteristic of the relative contributions of the borehole and the formation in the responses; and determining, for each depth, the respective values of the unknown for the borehole and for the formation, from the position on the cross-plot of the set of responses for that depth, with respect to the region.

  18. Studies of Fe/sup 2 +/. -->. Fe/sup 3 +/ transitions during the process of rock weathering by nuclear gamma-resonance spectroscopy

    SciTech Connect

    Vasil'ev, S.P.; Babanin, V.F.; Solov'ev, A.A.

    1986-11-01

    This paper presents a method for the mineral and weathering assessment of rocks and carbonaceous matter based in gamma spectroscopy and transitions between iron ions. The method is applied to rocks collected near the Teberda preserve. Four latitudinal bands of rocks parallel to the Greater Caucasus Ridge are identified in this territory. Isomer shift and hyperfine parameters of the Moessbauer spectra are given.

  19. ZnO film with ultra-low background electron concentration grown by plasma-assisted MBE using Mg film as the buffer layer

    SciTech Connect

    Chen, Mingming; Zhang, Quanlin; Su, Longxing; Su, Yuquan; Cao, Jiashi; Zhu, Yuan; Wu, Tianzhun; Gui, Xuchun; Yang, Chunlei; Xiang, Rong; Tang, Zikang

    2012-09-15

    Highlights: ► High quality ZnO film with ultra-low background electron concentration is grown by plasma-assisted molecular beam epitaxy using Mg film as a buffer layer. ► High resolution X-ray diffraction and photoluminescence (PL) spectroscopy indicate a high degree of crystallization. ► Hall measurement shows a carrier concentration as low as ∼10{sup 14} cm{sup −3}. ► The mechanism of the improved crystallinity is discussed in detail. -- Abstract: High quality ZnO epilayer with background electron concentration as low as 2.6 × 10{sup 14} cm{sup −3} was obtained by plasma-assisted MBE on c-sapphire using a thin Mg film as the buffer layer. High-resolution XRD measurement shows a sharp (0 0 2) peak with full width at half maximum (FWHM) of only 0.029°. Photoluminescence spectroscopy presents a weak defect-related near-edge emission. A metal–semiconductor–metal (MSM) typed photodetector based on the material demonstrates a response of ∼43 A/W under the bias of 1 V and an ON/OFF ratio of 10{sup 4}. This un-doped ZnO with ultra-low background electron concentration could be a promising starting material for p-type doping.

  20. Experimental setup for radon exposure and first diffusion studies using gamma spectroscopy

    NASA Astrophysics Data System (ADS)

    Maier, Andreas; van Beek, Patrick; Hellmund, Johannes; Durante, Marco; Schardt, Dieter; Kraft, Gerhard; Fournier, Claudia

    2015-11-01

    In order to measure the uptake and diffusion of 222Rn in biological material, an exposure chamber was constructed where cell cultures, biological tissues and mice can be exposed to 222Rn-activities similar to therapy conditions. After exposure, the material is transferred to a gamma spectrometer and the decay of 214Pb and 214Bi is analyzed. From the time kinetics of these decays the total amount of the initial 222Rn concentration can be calculated. In this paper the design and construction as well as first test measurements are reported.

  1. High resolution spectroscopy of two gamma-ray bursts in November 1978

    NASA Technical Reports Server (NTRS)

    Teegarden, B. J.; Cline, T. L.

    1979-01-01

    The first results from the ISSEE-3 radiatively colled germanium gamma ray burst spectrometer are presented. Spectra and time histories from two events on the 1978 November 4 and 1978 November 19 are given. A significant difference in the continuum spectra for the two events was observed. Evidence is presented for two spectral features in the features in the November 19 events, a broad one at approximately 420 key KeV and a narrower one at 740 KeV with a suggestion of an accompanying high energy tail.

  2. Fourier transform infrared photoacoustic spectroscopy of pyridine adsorbed on silica-alumina and. gamma. -alumina

    SciTech Connect

    Riseman, S.M.; Massoth, F.E.; Dhar, G.M.; Eyring, E.M.

    1982-05-13

    Relative numbers of Bronsted acid to Lewis acid sites on silica-alumina have been determined photoacoustically by an infrared analysis of chemisorbed pyridine compared to similar adsorption of ..gamma..-alumina that has only Lewis sites. Results are similar to those obtained by earlier IR transmission studies that suggested the use of framework vibrations of silica as an internal reference standard. The 20% coverage of the silica-alumina surface by pyridine adsorbed at Bronsted sites found photoacoustically is in good agreement with a previous value of 17% estimated from transmission spectroscopic data. Reproducibility of the photoacoustic measurements is excellent.

  3. High-resolution spectroscopy of two gamma-ray bursts in 1978 November

    NASA Technical Reports Server (NTRS)

    Teegarden, B. J.; Cline, T. L.

    1980-01-01

    The first results from the ISEE 3 radiatively cooled germanium gamma-ray burst spectrometer are presented. Spectra and time histories from two events on 1978 November 4 and 19 are given. A significant difference in the continuum spectra for the two events was observed. Evidence is presented for two spectral features in the November 19 event, a broad one at about 420 keV and a narrower one at about 740 keV with a suggestion of an accompanying high-energy tail.

  4. Continuous versus pulse neutron induced gamma spectroscopy for soil carbon analysis.

    PubMed

    Kavetskiy, A; Yakubova, G; Torbert, H A; Prior, S A

    2015-02-01

    Neutron induced gamma spectra analysis (NGA) provides a means of measuring carbon in large soil volumes without destructive sampling. Calibration of the NGA system must account for system background and the interference of other nuclei on the carbon peak at 4.43 MeV. Accounting for these factors produced measurements in agreement with theoretical considerations. The continuous NGA mode was twice as fast and just as accurate as the pulse mode, thus this mode was preferable for routine soil carbon analysis. PMID:25497322

  5. ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy.

    PubMed

    Ji, J; Colosimo, A M; Anwand, W; Boatner, L A; Wagner, A; Stepanov, P S; Trinh, T T; Liedke, M O; Krause-Rehberg, R; Cowan, T E; Selim, F A

    2016-01-01

    The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials. PMID:27550235

  6. Identification of gamma-ray irradiated medicinal herbs using pulsed photostimulated luminescence, thermoluminescence, and electron spin resonance spectroscopy.

    PubMed

    Pal, Sukdeb; Kim, Byeong Keun; Kim, Won Young; Kim, Min Jung; Ki, Hyeon A; Lee, Kyeong-Hee; Kang, Woo Suk; Kang, In Ho; Kang, Shin Jung; Song, Joon Myong

    2009-08-01

    Dried herbal samples consisting of root, rhizome, cortex, fruit, peel, flower, spike, ramulus, folium, and whole plant of 20 different medicinal herbs were investigated using pulsed photostimulated luminescence (PPSL), thermoluminescence (TL), and electron spin resonance spectroscopy (ESR) to identify gamma-ray irradiation treatment. Samples were irradiated at 0-50 kGy using a 60Co irradiator. PPSL measurement was applied as a rapid screening method. Control samples of 19 different herbs had photon counts less than the lower threshold value (700 counts 60 s(-1)). The photon counts of non-irradiated clematidis radix and irradiated evodia and gardenia fruits were between the lower and upper threshold values (700-5,000 counts 60 s(-1)). TL ratios, i.e., integrated areas of the first glow (TL1)/the second glow (TL2), were found to be less than 0.1 in all non-irradiated samples and higher than 0.1 in irradiated ones providing definite proof of radiation treatment. ESR spectroscopy was applied as an alternative rapid method. In most of the irradiated samples, mainly radiation-induced cellulosic, sugar, and relatively complicated carbohydrate radical ESR signals were detected. No radiation-specific ESR signal, except one intense singlet, was observed for irradiated scrophularia and scutellaria root and artemisiae argyi folium. PMID:19529925

  7. ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy

    PubMed Central

    Ji, J.; Colosimo, A. M.; Anwand, W.; Boatner, L. A.; Wagner, A.; Stepanov, P. S.; Trinh, T. T.; Liedke, M. O.; Krause-Rehberg, R.; Cowan, T. E.; Selim, F. A.

    2016-01-01

    The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials. PMID:27550235

  8. ZnO Luminescence and scintillation studied via photoexcitation, x-ray excitation, and gamma-induced positron spectroscopy"

    SciTech Connect

    Ji, C; Colosimo, A; Anwand, W; Boatner, Lynn A; Wagner, A; Stepanov, P S; Trinh, t t; Liedke, m o; Krause-Rehberg, R; Cowan, T E; Selim, F. A.

    2016-01-01

    Luminescence and scintillation in ZnO single crystals were measured by photoluminescence and X-ray-induced luminescence (XRIL). XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. The origin of green emission, the dominant trap emission in ZnO, was investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials or the surroundings. The measurements showed the absence of positron traps in the crystals and yielded a bulk positron lifetime value that is in complete agreement with the predicted theoretical value = thereby confirming the advantage of the GIPS method. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE.

  9. ZnO Luminescence and scintillation studied via photoexcitation, x-ray excitation, and gamma-induced positron spectroscopy"

    DOE PAGESBeta

    Ji, C; Colosimo, A; Anwand, W; Boatner, Lynn A; Wagner, A; Stepanov, P S; Trinh, t t; Liedke, m o; Krause-Rehberg, R; Cowan, T E; et al

    2016-01-01

    Luminescence and scintillation in ZnO single crystals were measured by photoluminescence and X-ray-induced luminescence (XRIL). XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. The origin of green emission, the dominant trap emission in ZnO, was investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials or the surroundings. The measurements showed the absence of positron traps in the crystalsmore » and yielded a bulk positron lifetime value that is in complete agreement with the predicted theoretical value = thereby confirming the advantage of the GIPS method. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE.« less

  10. High-resolution imaging gamma-ray spectroscopy with externally segmented germanium detectors

    NASA Technical Reports Server (NTRS)

    Callas, J. L.; Mahoney, W. A.; Varnell, L. S.; Wheaton, W. A.

    1993-01-01

    Externally segmented germanium detectors promise a breakthrough in gamma-ray imaging capabilities while retaining the superb energy resolution of germanium spectrometers. An angular resolution of 0.2 deg becomes practical by combining position-sensitive germanium detectors having a segment thickness of a few millimeters with a one-dimensional coded aperture located about a meter from the detectors. Correspondingly higher angular resolutions are possible with larger separations between the detectors and the coded aperture. Two-dimensional images can be obtained by rotating the instrument. Although the basic concept is similar to optical or X-ray coded-aperture imaging techniques, several complicating effects arise because of the penetrating nature of gamma rays. The complications include partial transmission through the coded aperture elements, Compton scattering in the germanium detectors, and high background count rates. Extensive electron-photon Monte Carlo modeling of a realistic detector/coded-aperture/collimator system has been performed. Results show that these complicating effects can be characterized and accounted for with no significant loss in instrument sensitivity.

  11. gamma-ray spectroscopy of neutron-rich {sup 40}S

    SciTech Connect

    Wang, Z. M.; Chapman, R.; Liang, X.; Burns, M.; Hodsdon, A.; Keyes, K.; Kumar, V.; Papenberg, A.; Smith, J. F.; Spohr, K. M.; Haas, F.; Caurier, E.; Curien, D.; Nowacki, F.; Azaiez, F.; Ibrahim, F.; Verney, D.; Behera, B. R.; Corradi, L.; Fioretto, E.

    2010-05-15

    Yrast states up to (6{sup +}) in the neutron-rich {sup 40}S nucleus have been studied using binary grazing reactions produced by the interaction of a 215 MeV beam of {sup 36}S ions with a thin {sup 208}Pb target. The novel experimental setup that combines the large acceptance magnetic spectrometer, PRISMA, and the high-efficiency gamma-ray detection array, CLARA, was used. A new gamma-ray transition at an energy of 1572 keV was observed and tentatively assigned to the (6{sup +})->(4{sup +}) transition. A comparison of experimental observations and the results of large-scale 0(Planck constant/2pi)omega sd-pf shell-model calculations indicates that one- and two-proton excitations from the 2s{sub 1/2} to the 1d{sub 3/2} orbitals play an important role in reproducing the {sup 40}S yrast level structure and the published B(E2;0{sub g.s.}{sup +}->2{sub 1}{sup +}) value. The structure of the yrast states of the even-A isotopes of sulfur is interpreted in terms of the configurations of valence protons and neutrons within the context of large-scale 0(Planck constant/2pi)omega sd-pf shell-model calculations.

  12. GERDA phase II detectors: Behind the production and characterisation at low background conditions

    NASA Astrophysics Data System (ADS)

    Maneschg, Werner; Gerda Collaboration

    2013-08-01

    The low background GERmanium Detector Array (GERDA) at Laboratori Nazionali del Gran Sasso (LNGS) is designed to search for the rare neutrinoless double beta decay (0νββ) in 76Ge. Bare germanium diodes are operated in liquid argon which is used as coolant, as passive and soon active as well shield against external radiation. Currently, Phase I of the experiment is running using ˜15 kg of co-axial High Purity Germanium diodes. In order to increase the sensitivity of the experiment 30 Broad Energy Germanium (BEGe) diodes will be added within 2013. This presentation reviews the production chain of the new BEGe detectors from isotopic enrichment to diode production and testing. As demonstrated all steps were carefully planned in order to minimize the exposure of the enriched germanium to cosmic radiation. Following this premise, acceptance and characterisation measurement of the newly produced diodes have been performed within the HEROICA project in the Belgian underground laboratory HADES close to the diode manufacturer. The test program and the results from a subset of the recently terminated GERDA Phase II BEGe survey will be presented.

  13. A 220Rn source for the calibration of low-background experiments

    NASA Astrophysics Data System (ADS)

    Lang, R. F.; Brown, A.; Brown, E.; Cervantes, M.; Macmullin, S.; Masson, D.; Schreiner, J.; Simgen, H.

    2016-04-01

    We characterize two 40 kBq sources of electrodeposited 228Th for use in low-background experiments. The sources efficiently emanate 220Rn, a noble gas that can diffuse in a detector volume. 220Rn and its daughter isotopes produce α-, β-, and γ-radiation, which may used to calibrate a variety of detector responses and features, before decaying completely in only a few days. We perform various tests to place limits on the release of other long-lived isotopes. In particular, we find an emanation of < 0.008 atoms/min/kBq (90% CL) for 228Th and (1.53 ± 0.04) atoms/min/kBq for 224Ra. The sources lend themselves in particular to the calibration of detectors employing liquid noble elements such as argon and xenon. With the source mounted in a noble gas system, we demonstrate that filters are highly efficient in reducing the activity of these longer-lived isotopes further. We thus confirm the suitability of these sources even for use in next-generation experiments, such as XENON1T/XENONnT, LZ, and nEXO.

  14. The Majorana Low-noise Low-background Front-end Electronics

    NASA Astrophysics Data System (ADS)

    Abgrall, N.; Aguayo, E.; Avignone, F. T.; Barabash, A. S.; Bertrand, F. E.; Boswell, M.; Brudanin, V.; Busch, M.; Byram, D.; Caldwell, A. S.; Chan, Y.-D.; Christofferson, C. D.; Combs, D. C.; Cuesta, C.; Detwiler, J. A.; Doe, P. J.; Efremenko, Yu.; Egorov, V.; Ejiri, H.; Elliott, S. R.; Fast, J. E.; Finnerty, P.; Fraenkle, F. M.; Galindo-Uribarri, A.; Giovanetti, G. K.; Goett, J.; Green, M. P.; Gruszko, J.; Guiseppe, V. E.; Gusev, K.; Hallin, A. L.; Hazama, R.; Hegai, A.; Henning, R.; Hoppe, E. W.; Howard, S.; Howe, M. A.; Keeter, K. J.; Kidd, M. F.; Kochetov, O.; Konovalov, S. I.; Kouzes, R. T.; LaFerriere, B. D.; Leon, J.; Leviner, L. E.; Loach, J. C.; MacMullin, J.; MacMullin, S.; Martin, R. D.; Meijer, S.; Mertens, S.; Nomachi, M.; Orrell, J. L.; O'Shaughnessy, C.; Overman, N. R.; Phillips, D. G.; Poon, A. W. P.; Pushkin, K.; Radford, D. C.; Rager, J.; Rielage, K.; Robertson, R. G. H.; Romero-Romero, E.; Ronquest, M. C.; Schubert, A. G.; Shanks, B.; Shima, T.; Shirchenko, M.; Snavely, K. J.; Snyder, N.; Suriano, A. M.; Thompson, J.; Timkin, V.; Tornow, W.; Trimble, J. E.; Varner, R. L.; Vasilyev, S.; Vetter, K.; Vorren, K.; White, B. R.; Wilkerson, J. F.; Wiseman, C.; Xu, W.; Yakushev, E.; Young, A. R.; Yu, C.-H.; Yumatov, V.

    The MAJORANA DEMONSTRATOR will search for the neutrinoless double beta decay (ββ(0ν)) of the isotope 76Ge with a mixed array of enriched and natural germanium detectors. In view of the next generation of tonne-scale germanium-based ββ(0ν)-decay searches, a major goal of the MAJORANA DEMONSTRATOR is to demonstrate a path forward to achieving a background rate at or below 1 cnt/(ROI-t-y) in the 4 keV region of interest (ROI) around the 2039-keV Q-value of the 76Ge ββ(0ν)-decay. Such a requirement on the background level significantly constrains the design of the readout electronics, which is further driven by noise and energy resolution performances. We present here the low-noise low- background front-end electronics developed for the low-capacitance p-type point contact (P-PC) germanium detectors of the MAJORANA DEMONSTRATOR. This resistive-feedback front-end, specifically designed to have low mass, is fabricated on a radioassayed fused-silica substrate where the feedback resistor consists of a sputtered thin film of high purity amorphous germanium and the feedback capacitor is based on the capacitance between gold conductive traces.

  15. Ship Effect Neutron Measurements And Impacts On Low-Background Experiments

    SciTech Connect

    Aguayo Navarrete, Estanislao; Kouzes, Richard T.; Siciliano, Edward R.

    2013-10-01

    The primary particles entering the upper atmosphere as cosmic rays create showers in the atmosphere that include a broad spectrum of secondary neutrons, muons and protons. These cosmic-ray secondaries interact with materials at the surface of the Earth, yielding prompt backgrounds in radiation detection systems, as well as inducing long-lived activities through spallation events, dominated by the higher-energy neutron secondaries. For historical reasons, the multiple neutrons produced in spallation cascade events are referred to as “ship effect” neutrons. Quantifying the background from cosmic ray induced activities is important to low-background experiments, such as neutrino-less double beta decay. Since direct measurements of the effects of shielding on the cosmic-ray neutron spectrum are not available, Monte Carlo modeling is used to compute such effects. However, there are large uncertainties (orders of magnitude) in the possible cross-section libraries and the cosmic-ray neutron spectrum for the energy range needed in such calculations. The measurements reported here were initiated to validate results from Monte Carlo models through experimental measurements in order to provide some confidence in the model results. The results indicate that the models provide the correct trends of neutron production with increasing density, but there is substantial disagreement between the model and experimental results for the lower-density materials of Al, Fe and Cu.

  16. The Majorana low-noise low-background front-end electronics

    DOE PAGESBeta

    Abgrall, N.; Aguayo, E.; Avignone, III, F. T.; Barabash, A. S.; Bertrand, F. E.; Boswell, M.; Brudanin, V.; Busch, M.; Byram, D.; Caldwell, A. S.; et al

    2015-03-24

    The Majorana Demonstrator will search for the neutrinoless double beta decay (ββ(0ν)) of the isotope ⁷⁶Ge with a mixed array of enriched and natural germanium detectors. In view of the next generation of tonne-scale germanium-based ββ(0ν)-decay searches, a major goal of the Majorana Demonstrator is to demonstrate a path forward to achieving a background rate at or below 1 cnt/(ROI-t-y) in the 4 keV region of interest (ROI) around the 2039-keV Q-value of the ⁷⁶Ge ββ(0ν)-decay. Such a requirement on the background level significantly constrains the design of the readout electronics, which is further driven by noise and energy resolutionmore » performances. We present here the low-noise low-background front-end electronics developed for the low-capacitance p-type point contact (P-PC) germanium detectors of the Majorana Demonstrator. This resistive-feedback front-end, specifically designed to have low mass, is fabricated on a radioassayed fused-silica substrate where the feedback resistor consists of a sputtered thin film of high purity amorphous germanium and the feedback capacitor is based on the capacitance between gold conductive traces.« less

  17. TREX-DM: a low background Micromegas-based TPC for low-mass WIMP detection

    NASA Astrophysics Data System (ADS)

    Iguaz, F. J.; Garza, J. G.; Aznar, F.; Castel, J. F.; Cebrián, S.; Dafni, T.; García, J. A.; Irastorza, I. G.; Lagraba, A.; Luzón, G.; Peiró, A.

    2016-05-01

    Dark Matter experiments are recently focusing their detection techniques in low-mass WIMPs, which requires the use of light elements and low energy threshold. In this context, we describe the TREX-DM experiment, a low background Micromegas-based TPC for low-mass WIMP detection. Its main goal is the operation of an active detection mass ~0.3 kg, with an energy threshold below 0.4 keVee and fully built with previously selected radiopure materials. This work describes the commissioning of the actual setup situated in a laboratory on surface and the updates needed for a possible physics run at the Canfranc Underground Laboratory (LSC) in 2016. A preliminary background model of TREX-DM is also presented, based on a Geant4 simulation, the simulation of the detector’s response and two discrimination methods: a conservative muon/electron and one based on a neutron source. Based on this background model, TREX-DM could be competitive in the search for low-mass WIMPs. In particular it could be sensitive, e.g., to the low-mass WIMP interpretation of the DAMA/LIBRA and other hints in a conservative scenario.

  18. The Majorana low background low noise front-end electronics

    NASA Astrophysics Data System (ADS)

    Abgrall, Nicolas

    2014-03-01

    The Majorana Demonstrator will search for the neutrinoless double beta decay (ββ (0 ν)) of 76Ge with a mixed array of enriched and natural germanium detectors. In view of the next generation of tonne-scale germanium-based ββ (0 ν)-decay searches that will probe the neutrino mass scale in the inverted-hierarchy region, a major goal of the experiment is to demonstrate a path forward to achieving a background rate at or below 1 cnt/(ROI-t-y) in the 4 keV region of interest (ROI) around the 2039-keV Q-value of the 76Ge ββ (0 ν)-decay. Such a requirement on the background level in conjunction with the best possible energy resolution to increase the signal-to-noise ratio in the ROI significantly constrain the readout electronics. We present here the low background low noise front-end electronics developed for the low-capacitance P-type point-contact (PPC) germanium detectors of the Majorana Demonstrator. This resistive-feedback front-end, specifically designed to have low mass, is fabricated on a radioactivity-assayed fused silica substrate where the feedback resistor consists of a sputtered thin film of high purity amorphous germanium and the feedback capacitor is based on the stray capacitance between circuit Au traces.

  19. The Majorana low-noise low-background front-end electronics

    SciTech Connect

    Abgrall, N.; Aguayo, E.; Avignone, III, F. T.; Barabash, A. S.; Bertrand, F. E.; Boswell, M.; Brudanin, V.; Busch, M.; Byram, D.; Caldwell, A. S.; Chan, Y. -D.; Christofferson, C. D.; Combs, D. C.; Cuesta, C.; Detwiler, J. A.; Doe, P. J.; Efremenko, Yu.; Egorov, V.; Ejiri, H.; Elliott, S. R.; Fast, J. E.; Finnerty, P.; Fraenkle, F. M.; Galindo-Uribarri, A.; Giovanetti, G. K.; Goett, J.; Green, M. P.; Gruszko, J.; Guiseppe, V. E.; Gusev, K.; Hallin, A. L.; Hazama, R.; Hegai, A.; Henning, R.; Hoppe, E. W.; Howard, S.; Howe, M. A.; Keeter, K. J.; Kidd, M. F.; Kochetov, O.; Konovalov, S. I.; Kouzes, R. T.; LaFerriere, B. D.; Leon, J.; Leviner, L. E.; Loach, J. C.; MacMullin, J.; MacMullin, S.; Martin, R. D.; Meijer, S.; Mertens, S.; Nomachi, M.; Orrell, J. L.; O'Shaughnessy, C.; Overman, N. R.; Phillips, II, D. G.; Poon, A. W.P.; Pushkin, K.; Radford, D. C.; Rager, J.; Rielage, K.; Robertson, R. G.H.; Romero-Romero, E.; Ronquest, M. C.; Schubert, A. G.; Shanks, B.; Shima, T.; Shirchenko, M.; Snavely, K. J.; Snyder, N.; Suriano, A. M.; Thompson, J.; Timkin, V.; Tornow, W.; Trimble, J. E.; Varner, R. L.; Vasilyev, S.; Vetter, K.; Vorren, K.; White, B. R.; Wilkerson, J. F.; Wiseman, C.; Xu, W.; Yakushev, E.; Young, A. R.; Yu, C. -H.; Yumatov, V.

    2015-03-24

    The Majorana Demonstrator will search for the neutrinoless double beta decay (ββ(0ν)) of the isotope ⁷⁶Ge with a mixed array of enriched and natural germanium detectors. In view of the next generation of tonne-scale germanium-based ββ(0ν)-decay searches, a major goal of the Majorana Demonstrator is to demonstrate a path forward to achieving a background rate at or below 1 cnt/(ROI-t-y) in the 4 keV region of interest (ROI) around the 2039-keV Q-value of the ⁷⁶Ge ββ(0ν)-decay. Such a requirement on the background level significantly constrains the design of the readout electronics, which is further driven by noise and energy resolution performances. We present here the low-noise low-background front-end electronics developed for the low-capacitance p-type point contact (P-PC) germanium detectors of the Majorana Demonstrator. This resistive-feedback front-end, specifically designed to have low mass, is fabricated on a radioassayed fused-silica substrate where the feedback resistor consists of a sputtered thin film of high purity amorphous germanium and the feedback capacitor is based on the capacitance between gold conductive traces.

  20. GERDA phase II detectors: Behind the production and characterisation at low background conditions

    SciTech Connect

    Maneschg, Werner; Collaboration: GERDA Collaboration; and others

    2013-08-08

    The low background GERmanium Detector Array (GERDA) at Laboratori Nazionali del Gran Sasso (LNGS) is designed to search for the rare neutrinoless double beta decay (0νββ) in {sup 76}Ge. Bare germanium diodes are operated in liquid argon which is used as coolant, as passive and soon active as well shield against external radiation. Currently, Phase I of the experiment is running using ∼15 kg of co-axial High Purity Germanium diodes. In order to increase the sensitivity of the experiment 30 Broad Energy Germanium (BEGe) diodes will be added within 2013. This presentation reviews the production chain of the new BEGe detectors from isotopic enrichment to diode production and testing. As demonstrated all steps were carefully planned in order to minimize the exposure of the enriched germanium to cosmic radiation. Following this premise, acceptance and characterisation measurement of the newly produced diodes have been performed within the HEROICA project in the Belgian underground laboratory HADES close to the diode manufacturer. The test program and the results from a subset of the recently terminated GERDA Phase II BEGe survey will be presented.

  1. Low Level Gamma Spectroscopy Measurements of Radium and Cesium in Lucerne (Medicago Sativa)

    NASA Astrophysics Data System (ADS)

    Fokapić, S.; Bikit, I.; Mrđa, D.; Vesković, M.; Slivka, J.; Mihaljev, Ž.; Ćupić, Ž.

    2007-04-01

    Nineteen years after Chernobyl nuclear accident, activity concentration of 137Cs still could be detected in food and soil samples in Central and Eastern Europe. In this paper radiation levels of radium and cesium in Lucerne will be presented. It is a perennial plant with a deep root system and it is widely grown throughout the world as forage for cattle. The samples of Lucerne were taken from twelve different locations in Vojvodina in the summer period July-September 2004. The samples were specially dried on the air and after that ground, powdered and mineralized by method of dry burning on the temperature of 450°C. Gamma spectrometry measurements of the ash were performed by means of actively shielded germanium detector with maximal background reduction. For cesium 137Cs 10 mBq/kg order of magnitude detection limits were achieved.

  2. Hard X-ray and gamma-ray imaging spectroscopy for the next solar maximum

    NASA Technical Reports Server (NTRS)

    Hudson, H. S.; Crannell, C. J.; Dennis, B. R.; Spicer, D. S.; Davis, J. M.; Hurford, G. J.; Lin, R. P.

    1990-01-01

    The objectives and principles are described of a single spectroscopic imaging package that can provide effective imaging in the hard X- and gamma-ray ranges. Called the High-Energy Solar Physics (HESP) mission instrument for solar investigation, the device is based on rotating modulation collimators with germanium semiconductor spectrometers. The instrument is planned to incorporate thick modulation plates, and the range of coverage is discussed. The optics permit the coverage of high-contrast hard X-ray images from small- and medium-sized flares with large signal-to-noise ratios. The detectors allow angular resolution of less than 1 arcsec, time resolution of less than 1 arcsec, and spectral resolution of about 1 keV. The HESP package is considered an effective and important instrument for investigating the high-energy solar events of the near-term future efficiently.

  3. Combined in-beam electron and {gamma}-ray spectroscopy of {sup 184,186}Hg

    SciTech Connect

    Scheck, M.; Butler, P. A.; Gaffney, L. P.; Carrol, R. J.; Cox, D.; Joss, D. T.; Herzberg, R.-D.; Page, R. D.; Papadakis, P.; Watkins, H. V.; Bree, N.; Huyse, M.; Van Duppen, P.; Grahn, T.; Greenlees, P. T.; Herzan, A.; Jakobsson, U.; Jones, P.; Julin, R.; Juutinen, S.

    2011-03-15

    By exploiting the SAGE spectrometer a simultaneous measurement of conversion electrons and {gamma} rays emitted in the de-excitation of excited levels in the neutron-deficient nuclei {sup 184,186}Hg was performed. The light Hg isotopes under investigation were produced using the 4n channels of the fusion-evaporation reactions of {sup 40}Ar and {sup 148,150}Sm. The measured K- and L-conversion electron ratios confirmed the stretched E2 nature of several transitions of the yrast bands in {sup 184,186}Hg. Additional information on the E0 component of the 2{sub 2}{sup +}{yields}2{sub 1}{sup +} transition in {sup 186}Hg was obtained.

  4. Early Results for the Geochemistry of Vesta from Gamma Ray and Neutron Spectroscopy

    NASA Astrophysics Data System (ADS)

    Prettyman, T. H.; Toplis, M. J.; Beck, A.; Feldman, W. C.; Forni, O.; Joy, S. P.; Lawrence, D. J.; McCoy, T. J.; McFadden, L. A.; McSween, H. Y.; Mittlefehldt, D. W.; Polanskey, C. A.; Rayman, M. D.; Raymond, C. A.; Reedy, R. C.; Russell, C. T.; Titus, T. N.

    2012-04-01

    In December of 2011, the Dawn spacecraft began low altitude mapping of asteroid 4 Vesta. At low altitudes, Dawn's Gamma Ray and Neutron Detector (GRaND)1 is sensitive to gamma rays and neutrons produced by cosmogenic nuclear reactions and radioactive decay occurring within the top few decimeters of the surface. From these nuclear emissions, the abundance of several major- and minor-elements, such as Fe, Mg, Si, K, and Th can be determined. Dawn will remain in a circular, polar low altitude mapping orbit (LAMO) for up to 16 weeks, enabling the determination of global maps with a spatial resolution of a few hundred kilometers. If the howardite, eucrite, and diogenite (HED) meteorites are representative of Vesta's crustal composition, then GRaND will be able to map the mixing ratios of whole-rock HED end-members, enabling the determination of the relative proportions of basaltic eucrite, cumulate eucrite, and diogenite as well as the proportions of mafic and plagioclase minerals. GRaND will also search for compositions not well-represented in the meteorite collection, such as evolved, K-rich lithologies, outcrops of olivine from Vesta's mantle or igneous intrusions in major impact basins, and possible source regions for the mesosiderites. GRaND will globally map the abundance of H, providing constraints on the delivery of H by solar wind and the infall of carbonaceous chondrite materials. The chemical data acquired by GRaND will be analyzed within the broader context of the Dawn mission, and will be compared to and integrated with maps of mafic mineral abundances, geologic provinces, gravity, shape and topography. The compositional data acquired by Dawn will provide a more complete picture of Vesta's thermal history and evolution, supplementing geochemical data from HED meteorite studies. GRaND's elemental specificity and depth sensitivity provides a unique view of a compositionally-diverse protoplanet, complementing data acquired by Dawn's Visible-Infrared (VIR

  5. Cesium hafnium chloride: A high light yield, non-hygroscopic cubic crystal scintillator for gamma spectroscopy

    SciTech Connect

    Burger, Arnold; Rowe, Emmanuel; Groza, Michael; Morales Figueroa, Kristle; Cherepy, Nerine J.; Beck, Patrick R.; Hunter, Steven; Payne, Stephen A.

    2015-10-05

    We report on the scintillation properties of Cs{sub 2}HfCl{sub 6} (cesium hafnium chloride or CHC) as an example of a little-known class of non-hygroscopic compounds having the generic cubic crystal structure of K{sub 2}PtCl{sub 6}. The crystals are easily growable from the melt using the Bridgman method with minimal precursor treatments or purification. CHC scintillation is centered at 400 nm, with a principal decay time of 4.37 μs and a light yield of up to 54 000 photons/MeV when measured using a silicon CCD photodetector. The light yield is the highest ever reported for an undoped crystal, and CHC also exhibits excellent light yield nonproportionality. These desirable properties allowed us to build and test CHC gamma-ray spectrometers providing energy resolution of 3.3% at 662 keV.

  6. Development of a Reference Database for Particle-Induced Gamma-ray Emission spectroscopy

    NASA Astrophysics Data System (ADS)

    Dimitriou, P.; Becker, H.-W.; Bogdanović-Radović, I.; Chiari, M.; Goncharov, A.; Jesus, A. P.; Kakuee, O.; Kiss, A. Z.; Lagoyannis, A.; Räisänen, J.; Strivay, D.; Zucchiatti, A.

    2016-03-01

    Particle-Induced Gamma-ray Emission (PIGE) is a powerful analytical technique that exploits the interactions of rapid charged particles with nuclei located near a sample surface to determine the composition and structure of the surface regions of solids by measurement of characteristic prompt γ rays. The potential for depth profiling of this technique has long been recognized, however, the implementation has been limited owing to insufficient knowledge of the physical data and lack of suitable user-friendly computer codes for the applications. Although a considerable body of published data exists in the nuclear physics literature for nuclear reaction cross sections with γ rays in the exit channel, there is no up-to-date, comprehensive compilation specifically dedicated to IBA applications. A number of PIGE cross-section data had already been uploaded to the Ion Beam Analysis Nuclear Data Library (IBANDL)

  7. Synthesis of bulk-size transparent gadolinium oxide–polymer nanocomposites for gamma ray spectroscopy

    PubMed Central

    Cai, Wen; Chen, Qi; Cherepy, Nerine; Dooraghi, Alex; Kishpaugh, David; Chatziioannou, Arion; Payne, Stephen; Xiang, Weidong

    2015-01-01

    Heavy element loaded polymer composites have long been proposed to detect high energy X- and γ-rays upon scintillation. The previously reported bulk composite scintillators have achieved limited success because of the diminished light output resulting from fluorescence quenching and opacity. We demonstrate the synthesis of a transparent nanocomposite comprising gadolinium oxide nanocrystals uniformly dispersed in bulk-size samples at a high loading content. The strategy to avoid luminescence quenching and opacity in the nanocomposite was successfully deployed, which led to the radioluminescence light yield of up to 27 000/MeV, about twice as much as standard commercial plastic scintillators. Nanocomposites monoliths (14 mm diameter by 3 mm thickness) with 31 wt% loading of nanocrystals generated a photoelectric peak for Cs-137 gamma (662 keV) with 11.4% energy resolution. PMID:26478816

  8. Gamma ray spectroscopy in astrophysics: An observational overview (50 keV-20 MeV)

    NASA Technical Reports Server (NTRS)

    Chupp, E. L.

    1978-01-01

    The observational status of gamma ray astronomy based on results reported prior to April 1978 is discussed. Specific line observations are reviewed from the Sun, the galactic plane, the Galactic Center region, the active Galaxy NGC 5128 (Cen A), the Crab Nebula region, and a transient source in the general direction of the anti-Galactic Center region. A statistical method is described which determines the relative probability that a given, reported observation is due to an external source as compared to a random fluctuation in the experimental background counting rate. Only a few of the many reported observations can be considered likely extraterrestrial observations of an extraterrestrial source made with a confidence level of 99%.

  9. Low Level Gamma Spectroscopy Measurements of Radium and Cesium in Lucerne (Medicago Sativa)

    SciTech Connect

    Fokapic, S.; Bikit, I.; Mrda, D.; Veskovic, M.; Slivka, J.; Mihaljev, Z.; Cupic, Z.

    2007-04-23

    Nineteen years after Chernobyl nuclear accident, activity concentration of 137Cs still could be detected in food and soil samples in Central and Eastern Europe. In this paper radiation levels of radium and cesium in Lucerne will be presented. It is a perennial plant with a deep root system and it is widely grown throughout the world as forage for cattle. The samples of Lucerne were taken from twelve different locations in Vojvodina in the summer period July-September 2004. The samples were specially dried on the air and after that ground, powdered and mineralized by method of dry burning on the temperature of 450 deg. C. Gamma spectrometry measurements of the ash were performed by means of actively shielded germanium detector with maximal background reduction. For cesium 137Cs 10 mBq/kg order of magnitude detection limits were achieved.

  10. Pixellated thallium bromide detectors for gamma-ray spectroscopy and imaging

    NASA Astrophysics Data System (ADS)

    Onodera, T.; Hitomi, K.; Shoji, T.; Hiratate, Y.

    2004-06-01

    Recently, pixellated semiconductor detectors exhibit high-energy resolution, which have been studied actively and fabricated from CdTe, CZT and HgI 2. Thallium bromide (TlBr) is a compound semiconductor characterized with its high atomic numbers (Tl=81, Br=35) and high density (7.56 g/cm 3). Thus, TlBr exhibits higher photon stopping power than other semiconductor materials used for radiation detector fabrication such as CdTe, CZT and HgI 2. The wide band gap of TlBr (2.68 eV) permits the detectors low-noise operation at around room temperature. Our studies made an effort to fabricate pixellated TlBr detectors had sufficient detection efficiency and good charge collection efficiency. In this study, pixellated TlBr detectors were fabricated from the crystals purified by the multipass zone-refining method and grown by the horizontal traveling molten zone (TMZ) method. The TlBr detector has a continuous cathode over one crystal surface and 3×3 pixellated anodes (0.57×0.57 mm 2 each) surrounded by a guard ring on the opposite surface. The electrodes were realized by vacuum evaporation of palladium through a shadow mask. Typical thickness of the detector was 2 mm. Spectrometric performance of the TlBr detectors was tested by irradiating them with 241Am (59.5 keV), 57Co (122 keV) and 137Cs (662 keV) gamma-ray sources at temperature of -20°C. Energy resolutions (FWHM) were measured to be 4.0, 6.0 and 9.7 keV for 59.5, 122 and 662 keV gamma-rays, respectively.

  11. Overview of in-beam gamma-ray spectroscopy at the RIBF

    NASA Astrophysics Data System (ADS)

    Doornenbal, Pieter

    2016-07-01

    At the Radioactive Isotope Beam Factory stable primary beams are accelerated up to 345 MeV/u and incident on a primary target to produce cocktail secondary beams with the fragment separator BigRIPS ranging from the lightest nuclei up to the lead region. For in-beam γ-ray spectroscopy, the secondary beams impinge on a reaction target at energies between 100 and 300 MeV/u. Reaction residues are identified with the ZeroDegree spectrometer and γ-rays detected with the NaI(Tl) based DALI2 array. This conference paper outlines the experimental setup and presents recent exemplary results.

  12. Design and performance of the Majorana low-noise low-background front-end electronics

    NASA Astrophysics Data System (ADS)

    Abgrall, Nicolas; Majorana Collaboration

    2014-09-01

    The Majorana Demonstrator will search for the neutrinoless double beta decay (ββ (0 ν)) of the isotope 76Ge. In view of the next generation of tonne-scale germanium-based ββ (0 ν)-decay searches, a major goal of the Majorana Demonstrator is to demonstrate a path forward to achieving a background rate at or below 1 cnt/(ROI-t-y) in the 4 keV region of interest (ROI) around the 2039-keV Q-value of the 76Ge ββ (0 ν)-decay. Such a requirement on the background level significantly constrains the design of the readout electronics which is further driven by noise performances. We present here the low-noise low-background front-end electronics developed for the low-capacitance P-type point-contact (PPC) germanium detectors of the Majorana Demonstrator. This resistive-feedback front-end, specifically designed to have low mass, is fabricated on a radioactivity-assayed fused silica substrate where the feedback resistor consists of a sputtered thin film of high purity amorphous germanium and the feedback capacitor is based on the capacitance between circuit Au traces. Performance studies of the front-end and associated back-end electronics in single and multi-detector systems, as well as on-site performances are reported. The Majorana Demonstrator will search for the neutrinoless double beta decay (ββ (0 ν)) of the isotope 76Ge. In view of the next generation of tonne-scale germanium-based ββ (0 ν)-decay searches, a major goal of the Majorana Demonstrator is to demonstrate a path forward to achieving a background rate at or below 1 cnt/(ROI-t-y) in the 4 keV region of interest (ROI) around the 2039-keV Q-value of the 76Ge ββ (0 ν)-decay. Such a requirement on the background level significantly constrains the design of the readout electronics which is further driven by noise performances. We present here the low-noise low-background front-end electronics developed for the low-capacitance P-type point-contact (PPC) germanium detectors of the Majorana

  13. Time Resolved Spectroscopy of SGR J1550-5418 Bursts Detected with Fermi/Gamma-Ray Burst Monitor

    NASA Astrophysics Data System (ADS)

    Younes, G.; Kouveliotou, C.; van der Horst, A. J.; Baring, M. G.; Granot, J.; Watts, A. L.; Bhat, P. N.; Collazzi, A.; Gehrels, N.; Gorgone, N.; Göğüş, E.; Gruber, D.; Grunblatt, S.; Huppenkothen, D.; Kaneko, Y.; von Kienlin, A.; van der Klis, M.; Lin, L.; Mcenery, J.; van Putten, T.; Wijers, R. A. M. J.

    2014-04-01

    We report on a time-resolved spectroscopy of the 63 brightest bursts of SGR J1550-5418, detected with the Fermi/Gamma-ray Burst Monitor during its 2008-2009 intense bursting episode. We performed spectral analysis down to 4 ms timescales to characterize the spectral evolution of the bursts. Using a Comptonized model, we find that the peak energy, E peak, anti-correlates with flux, while the low-energy photon index remains constant at ~ - 0.8 up to a flux limit F ≈ 10-5 erg s-1 cm-2. Above this flux value, the E peak-flux correlation changes sign, and the index positively correlates with the flux reaching ~1 at the highest fluxes. Using a two blackbody model, we find that the areas and fluxes of the two emitting regions correlate positively. Further, we study here for the first time the evolution of the temperatures and areas as a function of flux. We find that the area-kT relation follows the lines of constant luminosity at the lowest fluxes, R 2vpropkT -4, with a break at the higher fluxes (F > 10-5.5 erg s-1 cm-2). The area of the high-kT component increases with the flux while its temperature decreases, which we interpret as being due to an adiabatic cooling process. The area of the low-kT component, on the other hand, appears to saturate at the highest fluxes, toward R max ≈ 30 km. Assuming that crust quakes are responsible for soft gamma repeater (SGR) bursts and considering R max as the maximum radius of the emitting photon-pair plasma fireball, we relate this saturation radius to a minimum excitation radius of the magnetosphere, and we put a lower limit on the internal magnetic field of SGR J1550-5418, B int >~ 4.5 × 1015 G.

  14. Measuring fast neutrons with large liquid scintillation detector for ultra-low background experiments

    NASA Astrophysics Data System (ADS)

    Zhang, C.; Mei, D.-M.; Davis, P.; Woltman, B.; Gray, F.

    2013-11-01

    We developed a 12-liter volume neutron detector filled with the liquid scintillator EJ301 that measures neutrons in an underground laboratory where dark matter and neutrino experiments are located. The detector target is a cylindrical volume coated on the inside with reflective paint (95% reflectivity) that significantly increases the detector's light collection. We demonstrate several calibration techniques using point sources and cosmic-ray muons for energies up to 20 MeV for this large liquid scintillation detector. Neutron-gamma separation using pulse shape discrimination with a few MeV neutrons to hundreds of MeV neutrons is shown for the first time using a large liquid scintillator.

  15. SPECTROSCOPY OF THE LARGEST EVER {gamma}-RAY-SELECTED BL LAC SAMPLE

    SciTech Connect

    Shaw, Michael S.; Romani, Roger W.; Healey, Stephen E.; Michelson, Peter F.; Readhead, Anthony C. S.; Richards, Joseph L.; Max-Moerbeck, Walter; King, Oliver G.

    2013-02-20

    We report on spectroscopic observations covering most of the 475 BL Lacs in the second Fermi Large Area Telescope (LAT) catalog of active galactic nuclei (AGNs). Including archival measurements (correcting several erroneous literature values) we now have spectroscopic redshifts for 44% of the BL Lacs. We establish firm lower redshift limits via intervening absorption systems and statistical lower limits via searches for host galaxies for an additional 51% of the sample leaving only 5% of the BL Lacs unconstrained. The new redshifts raise the median spectroscopic z-tilde from 0.23 to 0.33 and include redshifts as large as z = 2.471. Spectroscopic redshift minima from intervening absorbers have z-tilde = 0.70, showing a substantial fraction at large z and arguing against strong negative evolution. We find that detected BL Lac hosts are bright ellipticals with black hole masses M {sub .} {approx} 10{sup 8.5} - 10{sup 9}, substantially larger than the mean of optical AGNs and LAT Flat Spectrum Radio Quasar samples. A slow increase in M {sub .} with z may be due to selection bias. We find that the power-law dominance of the optical spectrum extends to extreme values, but this does not strongly correlate with the {gamma}-ray properties, suggesting that strong beaming is the primary cause of the range in continuum dominance.

  16. Benchmark Gamma Spectroscopy Measurements of Uranium Hexafluoride in Aluminmum Pipe with a Sodium Iodide Detector

    SciTech Connect

    March-Leuba, Jose A; Uckan, Taner; Gunning, John E; Brukiewa, Patrick D; Upadhyaya, Belle R; Revis, Stephen M

    2010-01-01

    ) and an enrichment monitor (EM). Development of the FM is primarily the responsibility of Oak Ridge National Laboratory, and development of the EM is primarily the responsibility of Los Alamos National Laboratory. The FM will measure {sup 235}U mass flow rate by combining information from measuring the UF{sub 6} volumetric flow rate and the {sup 235}U density. The UF{sub 6} flow rate will be measured using characteristics of the process pumps used in product and tail UF{sub 6} header process lines of many GCEPs, and the {sup 235}U density will be measured using commercially available sodium iodide (NaI) gamma ray scintillation detectors. This report describes the calibration of the portion of the FM that measures the {sup 235}U density. Research has been performed to define a methodology and collect data necessary to perform this calibration without the need for plant declarations. The {sup 235}U density detector is a commercially available system (GammaRad made by Amptek, www.amptek.com) that contains the NaI crystal, photomultiplier tube, signal conditioning electronics, and a multichannel analyzer (MCA). Measurements were made with the detector system installed near four {sup 235}U sources. Two of the sources were made of solid uranium, and the other two were in the form of UF{sub 6} gas in aluminum piping. One of the UF{sub 6} gas sources was located at ORNL and the other at LANL. The ORNL source consisted of two pipe sections (schedule 40 aluminum pipe of 4-inch and 8-inch outside diameter) with 5.36% {sup 235}U enrichment, and the LANL source was a 4-inch schedule 40 aluminum pipe with 3.3% {sup 235}U enrichment. The configurations of the detector on these test sources, as well as on long straight pipe configurations expected to exist at GCEPs, were modeled using the computer code MCNP. The results of the MCNP calculations were used to define geometric correction factors between the test source and the GCEP application. Using these geometric correction factors

  17. Ultrahigh-Resolution {gamma}-Ray Spectroscopy of {sup 156}Gd: A Test of Tetrahedral Symmetry

    SciTech Connect

    Jentschel, M.; Krempel, J.; Urban, W.; Tonev, D.; Petkov, P.; Dudek, J.; Curien, D.; Lauss, B.; Angelis, G. de

    2010-06-04

    Tetrahedral symmetry in strongly interacting systems would establish a new class of quantum effects at subatomic scale. Excited states in {sup 156}Gd that could carry the information about the tetrahedral symmetry were populated in the {sup 155}Gd(n,{gamma}){sup 156}Gd reaction and studied using the GAMS4/5 Bragg spectrometers at the Institut Laue-Langevin. We have identified the 5{sub 1}{sup -{yields}}3{sub 1}{sup -} transition of 131.983(12) keV in {sup 156}Gd and determined its intensity to be 1.9(3)x10{sup -6} per neutron capture. The lifetime {tau}=220{sub -30}{sup +180}fs of the 5{sub 1}{sup -} state in {sup 156}Gd has been measured using the GRID technique. The resulting B(E2)=293{sub -134}{sup +61}Weisskopf unit rate of the 131.983 keV transition provides the intrinsic quadrupole moment of the 5{sub 1}{sup -} state in {sup 156}Gd to be Q{sub 0}=7.1{sub -1.6}{sup +0.7} b. This large value, comparable to the quadrupole moment of the ground state in {sup 156}Gd, gives strong evidence against tetrahedral symmetry in the lowest odd-spin, negative-parity band of {sup 156}Gd.

  18. Lu.sub.1-xI.sub.3:Ce.sub.x-a scintillator for gamma-ray spectroscopy and time-of-flight pet

    DOEpatents

    Shah, Kanai S.

    2008-02-12

    The present invention includes very fast scintillator materials including lutetium iodide doped with Cerium (Lu.sub.1-xI.sub.3:Ce.sub.x; LuI.sub.3:Ce). The LuI.sub.3 scintillator material has surprisingly good characteristics including high light output, high gamma-ray stopping efficiency, fast response, low cost, good proportionality, and minimal afterglow that the material is useful for gamma-ray spectroscopy, medical imaging, nuclear and high energy physics research, diffraction, non-destructive testing, nuclear treaty verification and safeguards, and geological exploration.

  19. Estimation of Cosmic Induced Contamination in Ultra-low Background Detector Materials

    SciTech Connect

    Aguayo Navarrete, Estanislao; Kouzes, Richard T.; Orrell, John L.; Berguson, Timothy J.; Greene, Austen T.

    2012-08-01

    Executive Summary This document presents the result of investigating a way to reliably determine cosmic induced backgrounds for ultra-low background materials. In particular, it focuses on those radioisotopes produced by the interactions with cosmic ray particles in the detector materials that act as a background for experiments looking for neutrinoless double beta decay. This investigation is motivated by the desire to determine background contributions from cosmic ray activation of the electroformed copper that is being used in the construction of the MAJORANA DEMONSTRATOR. The most important radioisotope produced in copper that contributes to the background budget is 60Co, which has the potential to deposit energy in the region of interest of this experiment. Cobalt-60 is produced via cosmic ray neutron collisions in the copper. This investigation aims to provide a method for determining whether or not the copper has been exposed to cosmic radiation beyond the threshold which the Majorana Project has established as the maximum exposure. This threshold is set by the Project as the expected contribution of this source of background to the overall background budget. One way to estimate cosmic ray neutron exposure of materials on the surface of the Earth is to relate it to the cosmic ray muon exposure. Muons are minimum-ionizing particles and the available technologies to detect muons are easier to implement than those to detect neutrons. We present the results of using a portable, ruggedized muon detector, the µ-Witness made by our research group, for determination of muon exposure of materials for the MAJORANA DEMONSTRATOR. From the muon flux measurement, this report presents a method to estimate equivalent sea-level exposure, and then infer the neutron exposure of the tracked material and thus the cosmogenic activation of the copper. This report combines measurements of the muon flux taken by the µ-Witness detector with Geant4 simulations in order to assure our

  20. AlSb photonic detectors for gamma-ray spectroscopy. Progress report, October 1994--August 1995

    SciTech Connect

    Becla, P.; Witt, A.F.

    1995-12-31

    Aluminum antimony (AlSb) is an indirect band gap semiconductor with Eg of about 1.62 eV at 300 K and about 1.75 eV at 77 K. This material, is extremely difficult to obtain in single crystal form because of the very high reactivity of aluminum with oxygen, and the high volatility of antimony. Moreover, molten AlSb reacts with nearly all crucible materials available. Since Welker`s first attempts in 1952, only very few different experimental approaches have been used to grow single crystals of AlSb, e.g. by Bridgman, Czochralski and MBE. All experimental results, however, indicate that many of the properties of AlSb, e.g. carrier concentration, electron-hole mobility and carrier life-time, differ significantly from the theoretically predicted values. The main objective of this research period has been to develop a method leading to improved crystallographic and electronic quality of AlSb crystals, making them more suitable for device applications. The research program was aimed along the following two directions: (1) study the growth of AlSb via Bridgman, Czochralski and THM techniques; (2) comprehensive characterization of grown material, related to the use of compounds for high energy gamma detectors. Variables in the growth study were growth temperature, equilibrium pressure, growth rate, doping, crucible material, seeding and encapsulation. The characterization study included crystallographic quality (grain size, etch pits, precipitates, inclusions), electronic quality (conductivity type, carrier concentration and mobility), optical properties (spectral absorption, photoconductivity, persistent absorption) and others (SIMS, EPR).

  1. Determination of low-level radioactivity in environmental samples by gamma spectroscopy at Argonne National Laboratory

    SciTech Connect

    Streets, W.E.; Heinrich, R.R.; Lamoureux, L.L.

    1988-01-01

    We currently have six Ge/Ge(Li) detectors that are being used for gamma counting of environmental samples (three with horizontal geometry, three with vertical geometry). The detectors were calibrated for close-geometry efficiency by counting standards in a set configuration (a height of 6.4 cm in a 4-oz. wide-mouthed Naglene bottle) immediately adjacent to the cryostat face. This configuration was chosen so that the standards would be symmetrical to the centers of both the horizontal and vertical detectors. Two solid standards were prepared by adding a known amount of Standard Reference Material NBL No. 6-A (Pitchblende) and NBL No. 7-A (Monazite Sand) to a blanked soil and mixing. Homogeneity of the standards was checked by counting each standard at each quadrant (on a horizontal detector). The final mixtures showed less than 1% deviation between the high and low quadrant counts. Two liquid secondary standards were prepared from stock solutions of /sup 137/Cs, /sup 131/I, and /sup 110m/Ag, which has been characterized as point sources using several detector efficiency curves. These efficiencies were determined using point source standards from the National Bureau of Standards (NBS) and International Atomic Energy Agency (IAEA). All standards had activity levels that allowed less than 1% counting statistics to be obtained on the major peaks (i.e., those with stronger branching ratio) within two hours. Analysis of the resulting data yield smooth efficiency curves for each of the six detectors. Although the standard compositions varied, solid and liquid, the densities were all approx. =1.0 g/cm/sup 3/. 3 refs.

  2. Neutron Spectroscopy of the Alpha and Gamma Forms of Nylon-6 Polymer

    NASA Astrophysics Data System (ADS)

    Papanek, Peter; Fischer, John E.; Murthy, N. S.

    1998-03-01

    The polyamide nylon-6 crystallizes in two different forms, α and γ, characterized by different chain conformations, and different arrangement of hydrogen bonds between chains. We have performed inelastic neutron scattering experiments to study the effects of H-bonding on lattice dynamics in both forms. Selectively deuterated and stretch oriented samples were used in order to identify the phonon modes and determine their polarization with respect to chain axes. Two complementary techniques, the filter-analyzer and time-of-flight (TOF) spectroscopy were employed. We have found that certain modes are similar in both α and γ fibers, however there are also significant differences in the 12--40 meV range, and in the frequencies of amide VI and amide VII modes. TOF spectra of both forms show broad low-frequency Boson peaks also at slightly different positions. The experimental results will be compared with semiempirical and ab initio calculations for a pair of chains at different relative orientations, and the relationship between the strength of H-bonds and amide vibrations will be discussed.

  3. ESR spectroscopy for detecting gamma-irradiated dried vegetables and estimating absorbed doses

    NASA Astrophysics Data System (ADS)

    Kwon, Joong-Ho; Chung, Hyung-Wook; Byun, Myung-Woo

    2000-03-01

    In view of an increasing demand for food irradiation technology, the development of a reliable means of detection for the control of irradiated foods has become necessary. Various vegetable food materials (dried cabbage, carrot, chunggyungchae, garlic, onion, and green onion), which can be legally irradiated in Korea, were subjected to a detection study using ESR spectroscopy. Correlation coefficients ( R2) between absorbed doses (2.5-15 kGy) and their corresponding ESR signals were identified from ESR signals. Pre-established threshold values were successfully applied to the detection of 54 coded unknown samples of dried clean vegetables ( chunggyungchae, Brassica camestris var. chinensis), both non-irradiated and irradiated. The ESR signals of irradiated chunggyungchae decreased over a longer storage time, however, even after 6 months of ambient storage, these signals were still distinguishable from those of non-irradiated samples. The most successful estimates of absorbed dose (5 and 8 kGy) were obtained immediately after irradiation using a quadratic fit with average values of 4.85 and 8.65 kGy being calculated.

  4. Segmented CdWO4 detector for low background experiments at DUSEL

    NASA Astrophysics Data System (ADS)

    Mei, Dongming; Sun, Yongchen; Day, Alyssa; Thomas, Keenan; Perevozchikov, Oleg

    2010-11-01

    We propose to develop a segmented CdWO4 scintillator array for detecting geo-neutrinos, neutrinoless double-beta, and dark matter. The detection of geo-neutrinos can shed light on the sources of the terrestrial heat flow, on the present composition, and on the origins of the Earth. The development of a new technique to detect geo-neutrinos through charge current antineutrino capture processes on ^106Cd is very interesting. This target allows us to detect all of geo-neutrinos from uranium, thorium, and potassium decays. When it is built, the detector can be also used to detect neutrinoless double-beta decay with ^116Cd. Both enriched ^106Cd and ^116Cd can be used to search for dark matter from the Universe. This paper will present RD results on the energy response of gamma-rays and neutrons from three small CdWO4 detectors.

  5. A Multiyear Light Curve of Scorpius X-1 Based on Compton Gamma Ray Observatory BATSE Spectroscopy Detector Observations

    NASA Astrophysics Data System (ADS)

    McNamara, B. J.; Harrison, T. E.; Mason, P. A.; Templeton, M.; Heikkila, C. W.; Buckley, T.; Galvan, E.; Silva, A.; Harmon, B. A.

    1998-06-01

    A multiyear light curve of the low mass X-ray binary, Scorpius X-1, is constructed based on the Compton Gamma Ray Observatory Burst and Transient Source Experiment (BATSE) Spectroscopy Detector (SD) data in the nominal energy range of 10-20 keV. A detailed discussion is given of the reduction process of the BATSE/SD data. Corrections to the SD measurements are made for off-axis pointings, spectral and bandpass changes, and differences in the eight SD sensitivities. The resulting 4.4 yr Sco X-1 SD light curve is characterized in terms of the timescales over which various types of emission changes occur. This light curve is then compared with Sco X-1 light curves obtained by Ariel 5, the BATSE Large Area Detectors (LADs), and the RXTE all-sky monitor (ASM). Coincident temporal coverage by the BATSE/SD and RXTE/ASM allows a direct comparison of the behavior of Sco X-1 over a range of high energies to be made. These ASM light curves are then used to discuss model constraints on the Sco X-1 system.

  6. Gamma irradiation and cellular damage in Kocuria rosea: investigation by one- and two-dimensional infrared spectroscopy.

    PubMed

    Melin, Anne-Marie; Perromat, Annie; Lorin, Chrystelle; Déléris, Gérard

    2002-12-15

    Fourier transform infrared (FT-IR) spectroscopy was used to investigate the radiation-induced effects on Kocuria rosea. Bacterial suspensions at the stationary phase were exposed to increasing doses of gamma radiation. In the region 1350-840cm(-1), assigned to phosphodiester backbone, nucleic acids, and sugar rings, the radical damaging effects were dose-dependent, with the first threshold at 2.75kGy and the second at 13.75kGy inducing more striking spectral variations. Postirradiation reincubation did not significantly affect the biomolecular response, except in the spectral range 1100-1000cm(-1). These observations suggest the occurrence of new phylogenetic characteristics for K. rosea following irradiation. Moreover, two-dimensional analysis was used to highlight correlated evolutions of molecular species as radical aggression increased. The results point to an evolutionary scheme during the time course of irradiation. Thus, one- and two-dimensional IR analyses are convenient means of investigating the metabolic events following oxidative stress generated by either chemical or physical agents. PMID:12464274

  7. Testing the Physical Mechanisms of Gamma-Ray Bursts with Multi-Instrument Time-Resolved Spectroscopy

    NASA Technical Reports Server (NTRS)

    Briggs, Michael S.; Preece, Robert E.

    2001-01-01

    We have continued the project of time-resolved spectral analyses of gamma-ray bursts observed jointly by the BATSE and the Wide-Field Camera on board BeppoSAX. We are making progress understanding the systematic differences between the two data sets. These data comprise the most important joint analysis set for our project. In several meetings, we have reported on metal efforts to understand the blackbody portion of the time series of spectra from GRB970111. Clearly, a fading thermal component can provide a 'seed' spectrum for Compton upscattering. It is very likely the X-ray excess that has been observed previously in BATSE data alone continues into the X-ray band observed by the WFC. We have also made progress in joint fitting of BATSE Large Area Detector and Spectroscopy Detector data with that of the Total Absorption Scintillation Calorimeter (TASC) of the EGRET experiment on CGRO. The TASC data are important to understanding the high-energy response of the BATSE data. We have produced time-sequences of spectra for two important GRB with data from both instruments. The Summer workshop on GRBs at the Aspen Center for Physics provided an opportunity for in-depth discussion of our on-going work. To aid our effort, we continue to make improvements in our spectral analysis software, RMFIT (rewritten from WINGSPAN).

  8. Sulfur Distribution on the Martian Surface Determined by Mars Odyssey Gamma Ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    McLennan, S. M.; Boynton, W. V.; Hahn, B. C.; Karunatillake, S.; Taylor, J.

    2009-12-01

    Understanding the sulfur cycle on Mars is central to evaluating the history of surficial aqueous processes on that planet. The sulfur-rich nature of Martian soils was recognized with the first chemical analyses returned by Viking landers, and confirmed by subsequent rovers Pathfinder, Spirit and Opportunity. Existence of regions on Mars with elevated sulfate mineralogy has also been demonstrated by various orbital IR spectrometers. Nevertheless, the global distribution of S on the Martian surface has remained unknown. For example, the recent Phoenix mission failed to unambiguously identify any sulfate minerals in north polar soils. After seven years of orbital measurements, the Mars Odyssey Gamma Ray Spectrometer (GRS) has obtained sufficient data to produce a statistically useful map of S distributions in the Martian near surface for low- to mid-latitudes (i.e., excluding high-latitude areas with H-enrichment: the so-called H-mask). The surface of Mars is characterized by elevated S, but varying from <1% to >3%, and with highest concentrations being found at low latitudes. Global average S content is approximately 2%, similar to average Martian soils analyzed to date. The overall distribution of S abundances, using 5°X5° bins, is characterized by a near-Gaussian distribution, similar to the distributions of other elements across the Martian surface measured by GRS. Sulfur exhibits highly scattered but statistically significant (at 95% confidence) positive bivariate correlations with both hydrogen and chlorine. In detail, the nature of these correlations differs for northern and southern hemispheres; for example the most extreme S values are mostly restricted to the northern hemisphere and correlation coefficients are larger in the south. For low latitudes, where occurrence of near surface ice is least likely (30°N to 30°S) the slope of the hydrogen - sulfur linear correlation can be interpreted as reflecting structural and/or bound water in near

  9. Studies on spin-trapped radicals in. gamma. -irradiated aqueous L-valine solutions by high-performance liquid chromatography and ESR spectroscopy

    SciTech Connect

    Makino, K.

    1980-05-01

    Short-lived radicals produced in ..gamma..-irradiated aqueous L-valine solution were investigated by the method of spin trapping and subsequently by means of high-performance liquid chromatography combined with ESR spectroscopy. Four spin adducts due to L-valine could be identified. Among them, even the diastereoisomeric spin adducts due to L-valine could be separated. In addition, the effect of pH on the change in the spectra of the diastereoisomers is discussed.

  10. Holdup Measures on an SRNL Mossbauer Spectroscopy Instrument

    SciTech Connect

    Dewberry, R.; Brown, T.; Salaymeh, S.

    2010-05-05

    Gamma-ray holdup measurements of a Mossbauer spectroscopy instrument are described and modeled. In the qualitative acquisitions obtained in a low background area of Savannah River National Laboratory, only Am-241 and Np-237 activity were observed. The Am-241 was known to be the instrumental activation source, while the Np-237 is clearly observed as a source of contamination internal to the instrument. The two sources of activity are modeled separately in two acquisition configurations using two separate modeling tools. The results agree well, demonstrating a content of (1980 {+-} 150) {mu}Ci Am-241 and (110 {+-} 50) {mu}Ci of Np-237.

  11. FY12 Final Report for PL10-Mod Separations-PD12: Electrochemically Modulated Separation of Plutonium from Dilute and Concentrated Dissolver Solutions for Analysis by Gamma Spectroscopy

    SciTech Connect

    Pratt, Sandra H.; Arrigo, Leah M.; Duckworth, Douglas C.; Cloutier, Janet M.; Breshears, Andrew T.; Schwantes, Jon M.

    2013-05-01

    Accurate and timely analysis of plutonium in spent nuclear fuel is critical in nuclear safeguards for detection of both protracted and rapid plutonium diversions. Gamma spectroscopy is a viable method for accurate and timely measurements of plutonium provided that the plutonium is well separated from the interfering fission and activation products present in spent nuclear fuel. Electrochemically modulated separation (EMS) is a method that has been used successfully to isolate picogram amounts of Pu from nitric acid matrices. With EMS, Pu adsorption may be turned “on” and “off” depending on the applied voltage, allowing for collection and stripping of Pu without the addition of chemical reagents. In this work, we have scaled up the EMS process to isolate microgram quantities of Pu from matrices encountered in spent nuclear fuel during reprocessing. Several challenges have been addressed including surface area limitations, radiolysis effects, electrochemical cell performance stability, and chemical interferences. After these challenges were resolved, 6 µg Pu was deposited in the electrochemical cell with approximately an 800-fold reduction of fission and activation product levels from a spent nuclear fuel sample. Modeling showed that these levels of Pu collection and interference reduction may not be sufficient for Pu detection by gamma spectroscopy. The main remaining challenges are to achieve a more complete Pu isolation and to deposit larger quantities of Pu for successful gamma analysis of Pu. If gamma analyses of Pu are successful, EMS will allow for accurate and timely on-site analysis for enhanced Pu safeguards.

  12. 207Pb(n,2n{gamma})206Pb Cross-Section Measurements by In-Beam Gamma-Ray Spectroscopy

    SciTech Connect

    Baumann, P.; Kerveno, M.; Rudolf, G.; Borcea, C.; Jericha, E.; Jokic, S.; Lukic, S.; Mihailescu, L. C.; Plompen, A. J. M.; Pavlik, A.

    2006-03-13

    207Pb(n,2n{gamma})206Pb cross section were measured for incident neutron energies between 6 and 20 MeV with the white neutron beam produced at GELINA. The {gamma}-ray production cross section for the main transition (803 keV, 2+{yields} 0+) in 206Pb is compared to results obtained at Los Alamos and to the TALYS and EMPIRE-II code predictions.

  13. Time resolved spectroscopy of SGR J1550–5418 bursts detected with Fermi/gamma-ray burst monitor

    SciTech Connect

    Younes, G.; Kouveliotou, C.; Collazzi, A.; Van der Horst, A. J.; Watts, A. L.; Huppenkothen, D.; Van der Klis, M.; Van Putten, T.; Baring, M. G.; Granot, J.; Bhat, P. N.; Gorgone, N.; Gehrels, N.; Mcenery, J.; Göğüş, E.; Kaneko, Y.; Lin, L.; Gruber, D.; Von Kienlin, A.; Grunblatt, S.; and others

    2014-04-10

    We report on a time-resolved spectroscopy of the 63 brightest bursts of SGR J1550–5418, detected with the Fermi/Gamma-ray Burst Monitor during its 2008-2009 intense bursting episode. We performed spectral analysis down to 4 ms timescales to characterize the spectral evolution of the bursts. Using a Comptonized model, we find that the peak energy, E {sub peak}, anti-correlates with flux, while the low-energy photon index remains constant at ∼ – 0.8 up to a flux limit F ≈ 10{sup –5} erg s{sup –1} cm{sup –2}. Above this flux value, the E {sub peak}–flux correlation changes sign, and the index positively correlates with the flux reaching ∼1 at the highest fluxes. Using a two blackbody model, we find that the areas and fluxes of the two emitting regions correlate positively. Further, we study here for the first time the evolution of the temperatures and areas as a function of flux. We find that the area–kT relation follows the lines of constant luminosity at the lowest fluxes, R {sup 2}∝kT {sup –4}, with a break at the higher fluxes (F > 10{sup –5.5} erg s{sup –1} cm{sup –2}). The area of the high-kT component increases with the flux while its temperature decreases, which we interpret as being due to an adiabatic cooling process. The area of the low-kT component, on the other hand, appears to saturate at the highest fluxes, toward R {sub max} ≈ 30 km. Assuming that crust quakes are responsible for soft gamma repeater (SGR) bursts and considering R {sub max} as the maximum radius of the emitting photon-pair plasma fireball, we relate this saturation radius to a minimum excitation radius of the magnetosphere, and we put a lower limit on the internal magnetic field of SGR J1550–5418, B {sub int} ≳ 4.5 × 10{sup 15} G.

  14. Infrared receivers for low background astronomy: Incoherent detectors and coherent devices from one micrometer to one millimeter

    NASA Technical Reports Server (NTRS)

    Boggess, N. W.; Greenberg, L. T.; Hauser, M. G.; Houck, J. R.; Low, F. J.; Mccreight, C. R.; Rank, D. M.; Richards, P. L.; Weiss, R.

    1979-01-01

    The status of incoherent detectors and coherent receivers over the infrared wavelength range from one micrometer to one millimeter is described. General principles of infrared receivers are included, and photon detectors, bolometers, coherent receivers, and important supporting technologies are discussed, with emphasis on their suitability for low background astronomical applications. Broad recommendations are presented and specific opportunities are identified for development of improved devices.

  15. Phase I Rinal Report: Ultra-Low Background Alpha Activity Counter

    SciTech Connect

    Warburton, W.K.

    2005-07-22

    In certain important physics experiments that search for rare-events, such as neutrino or double beta decay detections, it is critical to minimize the number of background events that arise from alpha particle emitted by the natural radioactivity in the materials used to construct the experiment. Similarly, the natural radioactivity in materials used to connect and package silicon microcircuits must also be minimized in order to eliminate ''soft errors'' caused by alpha particles depositing charges within the microcircuits and thereby changing their logic states. For these, and related reasons in the areas of environmental cleanup and nuclear materials tracking, there is a need that is important from commercial, scientific, and national security perspectives to develop an ultra-low background alpha counter that would be capable of measuring materials' alpha particle emissivity at rates well below 0.00001 alpha/cm{sup 2}/hour. This rate, which corresponds to 24 alpha particles per square meter per day, is essentially impossible to achieve with existing commercial instruments because the natural radioactivity of the materials used to construct even the best of these counters produces background rates at the 0.005 alpha/cm{sup 2}/hr level. Our company (XIA) had previously developed an instrument that uses electronic background suppression to operate at the 0.0005 0.005 alpha/cm{sup 2}/hr level. This patented technology sets up an electric field between a large planar sample and a large planar anode, and fills the gap with pure Nitrogen. An alpha particle entering the chamber ionizes the Nitrogen, producing a ''track'' of electrons, which drift to the anode in the electric field. Tracks close to the anode take less than 10 microseconds (us) to be collected, giving a preamplifier signal with a 10 us risetime. Tracks from the sample have to drift across the full anode-sample gap and produce a 35 us risetime signal. By analyzing the preamplifier signals with a digital

  16. First Year PIDDP Report on gamma-ray and x-ray spectroscopy: X-ray remote sensing and in situ spectroscopy for planetary exploration missions and gamma-ray remote sensing and in situ spectroscopy for planetary exploration missions

    NASA Technical Reports Server (NTRS)

    Mahdavi, M.; Giboni, K. L.; Vajda, S.; Schweitzer, J. S.; Truax, J. A.

    1994-01-01

    Detectors that will be used for planetary missions must have their responses calibrated in a reproducible manner. In addition, it is important to characterize a detector system at uneven portions of its life cycle, for example after exposure to different amounts of radiation. A calibration and response characterization facility has been constructed at Schlumberger-Doll Research for all types of gamma- and x-ray detectors that may be used for planetary measurement. This facility is currently being tested. Initial use is expected for the MARS 94 detectors. The facility will then also be available for calibrating other detectors as well as arrays of detectors such as the NEAR detector with its central Nal(TI) crystal surrounded with a large BGO crystal. Cadmium telluride detectors are investigated for applications in space explorations. These detectors show an energy resolution of 5 keV for the 122 keV 57Co line. Earlier reported polarization effects are not observed. The detectors can be used at temperatures up to 100 C, although with reduced energy resolution. The thickness of standard detectors is limited to 2 mm. These detectors become fully efficient at bias voltages above 200 V. Initial results for a 1 cm thick detector show that the quality of the material is inferior to the thinner standard detectors and hole trapping affects the pulse height. A detailed characterization of the detector is in progress. Prototypes of photomultipliers based on a Channel Electron Multiplier (CEM) are being built to study their performance. Such photomultipliers promise better timing characteristics and a higher dynamic range while being more compact and of lower in weight.

  17. A digital spectrometer approach to obtaining multiple time-resolved gamma-ray spectra for pulsed spectroscopy

    NASA Astrophysics Data System (ADS)

    Tan, H.; Mitra, S.; Fallu-Labruyere, A.; Hennig, W.; Chu, Y. X.; Wielopolski, L.; Warburton, W. K.

    2007-10-01

    Neutron-induced gamma-ray emission and its detection using a pulsed neutron generator system is an established analytical technique for quantitative multi-element analysis. Traditional gamma-ray spectrometers used for this type of analysis are normally operated either in coincidence mode - for counting prompt gamma-rays following inelastic neutron scattering (INS) events when the neutron generator is ON, or in anti-coincidence mode - for counting prompt gamma-rays from thermal neutron capture (TNC) processes when the neutron generator is OFF. We have developed a digital gamma-ray spectrometer for concurrently measuring both the INS and TNC gamma-rays using a 14 MeV pulsed neutron generator. The spectrometer separates the gamma-ray counts into two independent spectra together with two separate sets of counting statistics based on the external gate level. Because the TNC gamma-ray yields are time dependent, additional accuracy in analyzing the data can be obtained by acquiring multiple time-resolved gamma-ray spectra at finer time intervals than simply ON or OFF. For that purpose we are developing a multi-gating system that will allow gamma-ray spectra to be acquired concurrently in real time with up to 16 time slots. The conceptual system design is presented, especially focusing on considerations for tracking counting statistics in multiple time slots and on the placement of pulse heights into multiple spectra in real time.

  18. An Ultrasensitive Hot-Electron Bolometer for Low-Background SMM Applications

    NASA Technical Reports Server (NTRS)

    Olayaa, David; Wei, Jian; Pereverzev, Sergei; Karasik, Boris S.; Kawamura, Jonathan H.; McGrath, William R.; Sergeev, Andrei V.; Gershenson, Michael E.

    2006-01-01

    We are developing a hot-electron superconducting transition-edge sensor (TES) that is capable of counting THz photons and operates at T = 0.3K. The main driver for this work is moderate resolution spectroscopy (R approx. 1000) on the future space telescopes with cryogenically cooled (approx. 4 K) mirrors. The detectors for these telescopes must be background-limited with a noise equivalent power (NEP) approx. 10(exp -19)-10(exp -20) W/Hz(sup 1/2) over the range v = 0.3-10 THz. Above about 1 THz, the background photon arrival rate is expected to be approx. 10-100/s), and photon counting detectors may be preferable to an integrating type. We fabricated superconducting Ti nanosensors with a volume of approx. 3x10(exp -3) cubic microns on planar substrate and have measured the thermal conductance G to the thermal bath. A very low G = 4x10(exp -14) W/K, measured at 0.3 K, is due to the weak electron-phonon coupling in the material and the thermal isolation provided by superconducting Nb contacts. This low G corresponds to NEP(0.3K) = 3x10(exp -19) W/Hz(sup 1/2). This Hot-Electron Direct Detector (HEDD) is expected to have a sufficient energy resolution for detecting individual photons with v > 0.3 THz at 0.3 K. With the sensor time constant of a few microseconds, the dynamic range is approx. 50 dB.

  19. Low background techniques and experimental challenges for Borexino and its nylon vessels

    NASA Astrophysics Data System (ADS)

    Pocar, Andrea Pietro

    Borexino is an experiment for low energy (<1 MeV) solar neutrino spectroscopy approaching completion at the underground Gran Sasso laboratories in Italy. It is specifically designed to measure in real time the flux of mono-energetic {berillium} neutrinos produced by fusion reactions in the Sun. Its 300-ton liquid scintillator target is contained in an 8.5 meter diameter nylon inner vessel (IV) and is surrounded by 1000 tons of buffer fluid. A second, 11.5 meter diameter concentric nylon outer vessel (OV) around the IV serves as a barrier for radon emanated at the periphery of the detector. Borexino requires unprecedented low levels of radioactive impurities to be a success (˜1 background event/day in the central 100-tons of scintillator). The IV, which is in direct contact with the scintillator, also has to meet extremely stringent radioactive and cleanliness requirements. Intrinsic levels ˜10 -12 g/g for U and Th and ˜10-8 g/g for K are needed. The vessels, assembled in a clean room in Princeton, made of a 125 micron-thick membrane, need to be leak tight at the 10-2 cc/s and 1 cc/s level for the IV and OV respectively, and have to withstand mechanical stresses due to density differences and temperature gradients between the fluids they contain. Their requirements and assembly process are presented in detail. An upper limit on the inner vessel leak rate of 10-3 cc/s was measured. The performance of a matrix of light sources, placed on both vessels for monitoring its shape with digital cameras, is demonstrated. The problem of surface contamination by radon in the air is extensively addressed, strategies for minimizing it are analysed and the effectiveness of their application evaluated. In particular, an original radon filter based on vacuum swing adsorption on activated charcoal has been developed for use in connection with the clean room. Such a technique yielded radon abatement factors in excess of 104 in a small-scale prototype, and ˜100 in the final system

  20. Development of low background CsI(Tl) and NaI(Tl) crystals for WIMP search

    SciTech Connect

    Lee, Hyun Su

    2015-08-17

    We have developed low background CsI(Tl) and NaI(Tl) crystals to search for weakly interacting massive particles as well as to verify the origin of the annual modulation signal observed by the DAMA/LIBRA experiment. Extensive studies about the contamination mechanisim of {sup 137}Cs in CsI powder lead to the growth of ultra-low-background CsI(Tl) crystals. Similar approaches for NaI(Tl) crystals have been applied to reduce internal backgrounds to less than 0.5 counts/kg/day/keV. Status and understanding of backgrounds and background reduction in NaI(Tl) crystals will be discussed.

  1. KamLAND-PICO dark matter search project Low background test by highly radiopure NaI(Tl)

    NASA Astrophysics Data System (ADS)

    Fushimi, Kenichi; Ejiri, Hiroyasu; Hazama, Ryuta; Ikeda, Haruo; Imagawa, Kyoshiro; Inoue, Kunio; Kozlov, Alexandre; Orito, Reiko; Shima, Tatsushi; Takemoto, Yasuhiro; Umehara, Saori; Yasuda, Kensuke; KamLAND-PICO Collaboration

    2014-09-01

    KamLAND-PICO aims to search for WIMPs dark matter by means of highly radiopure NaI(Tl) scintillator. The impurities in NaI(Tl) has been successfully reduced by chemical processing of raw NaI(Tl) powder. The intensity of alpha ray was observed and the contamination in 210Pb has been dramatically reduced to about 60 μBq/kg. The present status of low background measurement will be reported.

  2. Defect Measurements of CdZnTe Detectors Using I-DLTS, TCT, I-V and Gamma-ray Spectroscopy

    SciTech Connect

    Gul,R.

    2008-08-11

    In this work we measured the crystal defect levels and tested the performance of CdZnTe detectors by diverse methodologies, viz., Current Deep Level Transient Spectroscopy (I-DLTS), Transient Current Technique (TCT), Current and Capacitance versus Voltage measurements (I-V and C-V), and gamma-ray spectroscopy. Two important characteristics of I-DLTS technique for advancing this research are (1) it is applicable for high-resistivity materials (>10{sup 6} {Omega}-cm), and, (2) the minimum temperature for measurements can be as low as 10 K. Such low-temperature capability is excellent for obtaining measurements at shallow levels. We acquired CdZnTe crystals grown by different techniques from two different vendors and characterized them for point defects and their response to photons. I-DLTS studies encompassed measuring the parameters of the defects, such as the energy levels in the band gap, the carrier capture cross-sections and their densities. The current induced by the laser-generated carriers and the charge collected (or number of electrons collected) were obtained using TCT that also provides the transport properties, such as the carrier life time and mobility of the detectors under study. The detector's electrical characteristics were explored, and its performance tested using I-V, C-V and gamma-ray spectroscopy.

  3. The efficiency calibration and development of environmental correction factors for an in situ high-resolution gamma spectroscopy well logging system

    SciTech Connect

    Giles, J.R.

    1996-05-01

    A Gamma Spectroscopy Logging System (GSLS) has been developed to study sub-surface radionuclide contamination. Absolute efficiency calibration of the GSLS was performed using simple cylindrical borehole geometry. The calibration source incorporated naturally occurring radioactive material (NORM) that emitted photons ranging from 186-keV to 2,614-keV. More complex borehole geometries were modeled using commercially available shielding software. A linear relationship was found between increasing source thickness and relative photon fluence rates at the detector. Examination of varying porosity and moisture content showed that as porosity increases, relative photon fluence rates increase linearly for all energies. Attenuation effects due to iron, water, PVC, and concrete cylindrical shields were found to agree with previous studies. Regression analyses produced energy-dependent equations for efficiency corrections applicable to spectral gamma-ray well logs collected under non-standard borehole conditions.

  4. Lu.sub.1-xI.sub.3:Ce.sub.x--a scintillator for gamma ray spectroscopy and time-of-flight PET

    DOEpatents

    Shah, Kanai S.

    2007-02-06

    The present invention concerns very fast scintillator materials comprising lutetium iodide doped with Cerium (Lu.sub.1-xI.sub.3:Ce.sub.x; LuI.sub.3:Ce). The LuI.sub.3 scintillator material has surprisingly good characteristics including high light output, high gamma ray stopping efficiency, fast response, low cost, good proportionality, and minimal afterglow that the material is useful for gamma ray spectroscopy, medical imaging, nuclear and high energy physics research, diffraction, non-destructive testing, nuclear treaty verification and safeguards, and geological exploration. The timing resolution of the scintillators of the present invention provide compositions capable of resolving the position of an annihilation event within a portion of a human body cross-section.

  5. GEMINI SPECTROSCOPY OF THE SHORT-HARD GAMMA-RAY BURST GRB 130603B AFTERGLOW AND HOST GALAXY

    SciTech Connect

    Cucchiara, A.; Prochaska, J. X.; Werk, J.; Cenko, S. B.; Cardwell, A.; Turner, J.; Bloom, J. S.; Cobb, B. E.

    2013-11-10

    We present early optical photometry and spectroscopy of the afterglow and host galaxy of the bright short-duration gamma-ray burst GRB 130603B discovered by the Swift satellite. Using our Target of Opportunity program on the Gemini South telescope, our prompt optical spectra reveal a strong trace from the afterglow superimposed on continuum and emission lines from the z = 0.3568 ± 0.0005 host galaxy. The combination of a relatively bright optical afterglow (r' = 21.52 at Δt = 8.4 hr), together with an observed offset of 0.''9 from the host nucleus (4.8 kpc projected distance at z = 0.3568), allow us to extract a relatively clean spectrum dominated by afterglow light. Furthermore, the spatially resolved spectrum allows us to constrain the properties of the explosion site directly, and compare these with the host galaxy nucleus, as well as other short-duration GRB host galaxies. We find that while the host is a relatively luminous (L∼0.8 L{sup *}{sub B}), star-forming (SFR = 1.84 M{sub ☉} yr{sup –1}) galaxy with almost solar metallicity, the spectrum of the afterglow exhibits weak Ca II absorption features but negligible emission features. The explosion site therefore lacks evidence of recent star formation, consistent with the relatively long delay time distribution expected in a compact binary merger scenario. The star formation rate (SFR; both in an absolute sense and normalized to the luminosity) and metallicity of the host are both consistent with the known sample of short-duration GRB hosts and with recent results which suggest GRB 130603B emission to be the product of the decay of radioactive species produced during the merging process of a neutron-star-neutron-star binary ({sup k}ilonova{sup )}. Ultimately, the discovery of more events similar to GRB 130603B and their rapid follow-up from 8 m class telescopes will open new opportunities for our understanding of the final stages of compact-objects binary systems and provide crucial information

  6. Radioactive Waste Characterization Strategies; Comparisons Between AK/PK, Dose to Curie Modeling, Gamma Spectroscopy, and Laboratory Analysis Methods- 12194

    SciTech Connect

    Singledecker, Steven J.; Jones, Scotty W.; Dorries, Alison M.; Henckel, George; Gruetzmacher, Kathleen M.

    2012-07-01

    In the coming fiscal years of potentially declining budgets, Department of Energy facilities such as the Los Alamos National Laboratory (LANL) will be looking to reduce the cost of radioactive waste characterization, management, and disposal processes. At the core of this cost reduction process will be choosing the most cost effective, efficient, and accurate methods of radioactive waste characterization. Central to every radioactive waste management program is an effective and accurate waste characterization program. Choosing between methods can determine what is classified as low level radioactive waste (LLRW), transuranic waste (TRU), waste that can be disposed of under an Authorized Release Limit (ARL), industrial waste, and waste that can be disposed of in municipal landfills. The cost benefits of an accurate radioactive waste characterization program cannot be overstated. In addition, inaccurate radioactive waste characterization of radioactive waste can result in the incorrect classification of radioactive waste leading to higher disposal costs, Department of Transportation (DOT) violations, Notice of Violations (NOVs) from Federal and State regulatory agencies, waste rejection from disposal facilities, loss of operational capabilities, and loss of disposal options. Any one of these events could result in the program that mischaracterized the waste losing its ability to perform it primary operational mission. Generators that produce radioactive waste have four characterization strategies at their disposal: - Acceptable Knowledge/Process Knowledge (AK/PK); - Indirect characterization using a software application or other dose to curie methodologies; - Non-Destructive Analysis (NDA) tools such as gamma spectroscopy; - Direct sampling (e.g. grab samples or Surface Contaminated Object smears) and laboratory analytical; Each method has specific advantages and disadvantages. This paper will evaluate each method detailing those advantages and disadvantages

  7. New Applications of Gamma Spectroscopy: Characterization Tools for D&D Process Development, Inventory Reduction Planning & Shipping, Safety Analysis & Facility Management During the Heavy Element Facility Risk Reduction Program

    SciTech Connect

    Mitchell, M; Anderson, B; Gray, L; Vellinger, R; West, M; Gaylord, R; Larson, J; Jones, G; Shingleton, J; Harris, L; Harward, N

    2006-01-23

    Novel applications of gamma ray spectroscopy for D&D process development, inventory reduction, safety analysis and facility management are discussed in this paper. These applications of gamma spectroscopy were developed and implemented during the Risk Reduction Program (RPP) to successfully downgrade the Heavy Element Facility (B251) at Lawrence Livermore National Laboratory (LLNL) from a Category II Nuclear Facility to a Radiological Facility. Non-destructive assay in general, gamma spectroscopy in particular, were found to be important tools in project management, work planning, and work control (''Expect the unexpected and confirm the expected''), minimizing worker dose, and resulted in significant safety improvements and operational efficiencies. Inventory reduction activities utilized gamma spectroscopy to identify and confirm isotopics of legacy inventory, ingrowth of daughter products and the presence of process impurities; quantify inventory; prioritize work activities for project management; and to supply information to satisfy shipper/receiver documentation requirements. D&D activities utilize in-situ gamma spectroscopy to identify and confirm isotopics of legacy contamination; quantify contamination levels and monitor the progress of decontamination efforts; and determine the point of diminishing returns in decontaminating enclosures and glove boxes containing high specific activity isotopes such as {sup 244}Cm and {sup 238}Pu. In-situ gamma spectroscopy provided quantitative comparisons of several decontamination techniques (e.g. TLC-free Stripcoat{trademark}, Radiac{trademark} wash, acid wash, scrubbing) and was used as a part of an iterative process to determine the appropriate level of decontamination and optimal cost to benefit ratio. Facility management followed a formal, rigorous process utilizing an independent, state certified, peer-reviewed gamma spectroscopy program, in conjunction with other characterization techniques, process knowledge, and

  8. Potential radionuclide emissions from stacks on the Hanford site, Part 2: Dose assessment methodology using portable low-resolution gamma spectroscopy

    SciTech Connect

    Barnett, J.M.

    1995-02-01

    In September 1992, the Westinghouse Hanford Company began developing an in situ measurement method to assess gamma radiation emanating from high-efficiency particulate air filters using portable low-resolution gamma spectroscopy. The purpose of the new method was to assess radioactive exhaust stack air emissions from empirical data rather than from theoretical models and to determine the potential unabated dose to an offsite theoretical maximally exposed individual. In accordance with Title 40, Code of Federal Regulations, Part 61, Subpart H, {open_quotes}National Emission Standards for Hazardous Air Pollutants{close_quotes}, stacks that have the potential to emit {ge} 1 {mu}Sv y{sup {minus}1} (0.1 mrem y{sup {minus}1}) to the maximally exposed individual are considered {open_quotes}major{close_quotes} and must meet the continuous monitoring requirements. After the method was tested and verified, the U.S. Environmental Protection Agency, Region 10, approved its use in June 1993. Of the 125 stacks operated by the Westinghouse Hanford Company, 22 were targeted for evaluation by this method, and 15 were assessed. (The method could not be applied at seven stacks because of excessive background radiation or because no gamma emitting particles appear in the emission stream.) The most significant result from this study was the redesignation of the T Plant main stack. The stack was assessed as being {open_quotes}minor{close_quotes}, and it now only requires periodic confirmatory measurements and meets federally imposed sampling requirements.

  9. Label-free fluorescence strategy for sensitive detection of adenosine triphosphate using a loop DNA probe with low background noise.

    PubMed

    Lin, Chunshui; Cai, Zhixiong; Wang, Yiru; Zhu, Zhi; Yang, Chaoyong James; Chen, Xi

    2014-07-15

    A simple, rapid, label-free, and ultrasensitive fluorescence strategy for adenosine triphosphate (ATP) detection was developed using a loop DNA probe with low background noise. In this strategy, a loop DNA probe, which is the substrate for both ligation and digestion enzyme reaction, was designed. SYBR green I (SG I), a double-stranded specific dye, was applied for the readout fluorescence signal. Exonuclease I (Exo I) and exonuclease III (Exo III), sequence-independent nucleases, were selected to digest the loop DNA probe in order to minimize the background fluorescence signal. As a result, in the absence of ATP, the loop DNA was completely digested by Exo I and Exo III, leading to low background fluorescence owing to the weak electrostatic interaction between SG I and mononucleotides. On the other hand, ATP induced the ligation of the nicking site, and the sealed loop DNA resisted the digestion of Exo I and ExoIII, resulting in a remarkable increase of fluorescence response. Upon background noise reduction, the sensitivity of the ATP determination was improved significantly, and the detection limitation was found to be 1.2 pM, which is much lower than that in almost all the previously reported methods. This strategy has promise for wide application in the determination of ATP. PMID:24983417

  10. {gamma}-ray Spectroscopy of Proton Drip-Line Nuclei in the A{approx}130 Region using SPIRAL beams

    SciTech Connect

    Stezowski, O.; Guinet, D.; Lautesse, Ph.; Meyer, M.; Redon, N.; Rosse, B.; Schmitt, Ch.; De France, G.; Bhattachasyya, S.; Mukherjee, G.

    2008-11-11

    A fusion-evaporation experiment has been performed with a SPIRAL {sup 76}Kr radioactive beam in order to study the deformation of rare-earth nuclei near the proton drip-line. The experimental setup consisted in the EXOGAM {gamma}-array, coupled to the light-charged particles (LCP) DIAMANT detector and to the VAMOS heavy-ion spectrometer. The difficulties inherent to such measurements are enlightened. The coupling between EXOGAM and DIAMANT has been used to decrease the huge background caused by the radioactivity of the beam. It further permits assigning new {gamma}-ray transitions to specific residual nuclei. A {gamma}-ray belonging to the {sup 130}Pm level scheme has thus been observed for the first time.

  11. First results of a simultaneous measurement of tritium and (14)C in an ultra-low-background proportional counter for environmental sources of methane.

    PubMed

    Mace, E K; Aalseth, C E; Day, A R; Hoppe, E W; Keillor, M E; Moran, J J; Panisko, M E; Seifert, A; Tatishvili, G; Williams, R M

    2016-05-01

    Simultaneous measurement of tritium and (14)C would provide an added tool for tracing organic compounds through environmental systems and is possible via beta energy spectroscopy of sample-derived methane in internal-source gas proportional counters. Since the mid-1960's atmospheric tritium and (14)C have fallen dramatically as the isotopic injections from aboveground nuclear testing have been diluted into the ocean and biosphere. In this work, the feasibility of simultaneous tritium and (14)C measurements via proportional counters is revisited in light of significant changes in both the atmospheric and biosphere isotopics and the development of new ultra-low-background gas proportional counting capabilities for small samples (roughly 50 cc methane). A Geant4 Monte Carlo model of a Pacific Northwest National Laboratory (PNNL) proportional counter response to tritium and (14)C is used to analyze small samples of two different methane sources to illustrate the range of applicability of contemporary simultaneous measurements and their limitations. Because the two methane sources examined were not sample size limited, we could compare the small-sample measurements performed at PNNL with analysis of larger samples performed at a commercial laboratory. These first results show that the dual-isotope simultaneous measurement is well matched for methane samples that are atmospheric or have an elevated source of tritium (i.e. landfill gas). However, for samples with low/modern tritium isotopics (rainwater), commercial separation and counting is a better fit. PMID:26990077

  12. a Quantitative Method for Analyzing Radioactive Nuclides in Infinite Composite Materials Using High-Resolution Gamma-Ray Spectroscopy.

    NASA Astrophysics Data System (ADS)

    Day, John Henry, Jr.

    1982-03-01

    A theory is formulated in which the concentration of a radionuclide uniformly distributed throughout an infinite medium is related to the photopeak count rate of a signature gamma ray acquired by a detector within the medium. The mass fraction of the i('th) radionuclide in the medium is given by f(,i) = W(,i)(psi)(,i) (E)/(lamda)(,i)I(,I)(E)K(E); where (psi)(,i)(E) and I(,i)(E) are the observed photopeak count rate and absolute intensity for a gamma-ray emission of energy E. (lamda)(,i) and W(,i) are the decay constant and isotopic mass, respectively. It is shown that the function K(E) is a source volume integration over(' )(epsilon)(E,R)B(E,R)exp( -(SIGMA)(mu)(E)r(R))/(VBAR)R(VBAR)('2) which depends on gamma-ray energy only. Values of the narrow-beam attenuation coefficient (mu) are known for many materials. However, several laboratory experiments are performed in order to obtain data from which to empirically determine the detector response function (epsilon)(E,R)(' )and the gamma-ray build -up-factor(' )B(E,R). Special experimental instrumentation for analyzing radionuclides in infinite composite materials using high -resolution gamma-ray spectrometry is introduced. A probe is constructed which contains a coaxial high-purity germanium crystal to detect the gamma rays, a cryostat to cool the crystal and electronic circuitry to process the signal from the detector. Laboratory models of natural formations are prepared using high-grade radioactive samples diluted with silicon dioxide to obtain the desired concentrations. Each model is sampled to obtain X-ray fluorescence, delayed neutron and fluorimetric analysis from independent laboratories to compare with results using the method presented in this work.

  13. Coupled multi-group neutron photon transport for the simulation of high-resolution gamma-ray spectroscopy applications

    SciTech Connect

    Burns, Kimberly A.

    2009-08-01

    The accurate and efficient simulation of coupled neutron-photon problems is necessary for several important radiation detection applications. Examples include the detection of nuclear threats concealed in cargo containers and prompt gamma neutron activation analysis for nondestructive determination of elemental composition of unknown samples.

  14. Initial characterization of unequal-length, low-background proportional counters for absolute gas-counting applications

    SciTech Connect

    Mace, E. K.; Aalseth, C. E.; Bonicalzi, R.; Day, A. R.; Fuller, E. S.; Hayes, J. C.; Hoppe, E. W.; LaFerriere, B. D.; Merriman, J. H.; Overman, C. T.; Seifert, A.; Williams, R. M.

    2013-08-08

    Characterization of two sets of custom unequal length proportional counters is underway at Pacific Northwest National Laboratory (PNNL). These detectors will be used in measurements to determine the absolute activity concentration of gaseous radionuclides (e.g., {sup 37}Ar). A set of three detectors has been fabricated based on previous PNNL ultra-low-background proportional counter designs and now operate in PNNL's shallow underground counting laboratory. A second set of four counters has also been fabricated using clean assembly of Oxygen-Free High-Conductivity copper components for use in a shielded above-ground counting laboratory. Characterization of both sets of detectors is underway with measurements of background rates, gas gain, and energy resolution. These results will be presented along with a shielding study for the above-ground cave.

  15. HDice, Highly-Polarized Low-Background Frozen-Spin HD Targets for CLAS experiments at Jefferson Lab

    SciTech Connect

    Wei, Xiangdong; Bass, Christopher; D'Angelo, Annalisa; Deur, Alexandre P.; Dezern, Gary L.; Ho, Dao Hoang; Kageya, Tsuneo; Khandaker, Mahbubul A,; Kashy, David H.; Laine, Vivien Eric; Lowry, Michael M.; O'Connell, Thomas Robert; Sandorfi, Andrew M.; Teachey, II, Robert W.; Whisnant, Charles Steven; Zarecky, Michael R.

    2012-12-01

    Large, portable frozen-spin HD (Deuterium-Hydride) targets have been developed for studying nucleon spin properties with low backgrounds. Protons and Deuterons in HD are polarized at low temperatures (~10mK) inside a vertical dilution refrigerator (Oxford Kelvinox-1000) containing a high magnetic field (up to 17T). The targets reach a frozen-spin state within a few months, after which they can be cold transferred to an In-Beam Cryostat (IBC). The IBC, a thin-walled dilution refrigerator operating either horizontally or vertically, is use with quasi-4{pi} detector systems in open geometries with minimal energy loss for exiting reaction products in nucleon structure experiments. The first application of this advanced target system has been used for Spin Sum Rule experiments at the LEGS facility in Brookhaven National Laboratory. An improved target production and handling system has been developed at Jefferson Lab for experiments with the CEBAF Large Acceptance Spectrometer, CLAS.

  16. Initial Characterization of Unequal-Length, Low-Background Proportional Counters for Absolute Gas-Counting Applications

    SciTech Connect

    Mace, Emily K.; Aalseth, Craig E.; Bonicalzi, Ricco; Day, Anthony R.; Fuller, Erin S.; Hayes, James C.; Hoppe, Eric W.; LaFerriere, Brian D.; Merriman, Jason H.; Overman, Cory T.; Seifert, Allen; Williams, Richard M.

    2013-08-31

    Abstract. Characterization of two sets of custom unequal length proportional counters is underway at Pacific Northwest National Laboratory (PNNL). These detectors will be used in measurements to determine the absolute activity concentration of gaseous radionuclides (e.g., 37Ar). A set of three detectors has been fabricated based on previous PNNL ultra-low-background proportional counters (ULBPC) designs and now operate in PNNL’s shallow underground counting laboratory. A second set of four counters has also been fabricated using clean assembly of OFHC copper components for use in an above-ground counting laboratory. Characterization of both sets of detectors is underway with measurements of background rates, gas gain, energy resolution, and shielding considerations. These results will be presented along with uncertainty estimates of future absolute gas counting measurements.

  17. Gamma-ray spectroscopy of the galactic center region: Confirmation of the time-variability of the positron annihilation line

    NASA Technical Reports Server (NTRS)

    Paciesas, W. S.; Cline, T. L.; Teegarden, B. J.; Tueller, J.; Durouchoux, P.; Hameury, J. M.

    1982-01-01

    The GSFC Low-Energy Gamma-Ray Spectrometer observed the region of the galactic center during a balloon flight from Alice Springs, Australia, on 1981 November 20. No significant excess over background was evident in the 511 keV annihilation line. A 98 percent confidence upper limit is derived for this line of 1.2 x .001 photons/sq. cm-s. Continuum emission was detected above 100 keV with a best-fitting power law spectrum.

  18. Incomplete-fusion reactions for {gamma}-ray spectroscopy: Application to the study of high-spin states in {sup 234}U

    SciTech Connect

    Lane, G. J.; Dracoulis, G. D.; Byrne, A. P.; McGoram, T. R.; Poletti, A. R.

    1999-09-02

    Incomplete-fusion reactions occur when breakup of the projectile results in only part of the beam particle fusing with the target, the remnant being emitted with an energy equivalent to the beam velocity. Such reactions have been demonstrated to populate slightly neutron-rich nuclei compared to conventional fusion-evaporation reactions, opening possibilities for the study of nuclei along the neutron-rich side of the line of stability. Results from a study of {sup 211}Po are presented to illustrate the use of incomplete-fusion reactions for {gamma}-ray spectroscopy. New results from a test-run which populated high-spin states in {sup 234}U via the {sup 232}Th({sup 9}Be,{alpha}3n) reaction are also presented. An interesting feature of the latter reaction is that the high fission probabilities for the compound nuclei which follow complete fusion, results in the residues from incomplete fusion forming the dominant residue channels.

  19. Copper doping of ZnO crystals by transmutation of {sup 64}Zn to {sup 65}Cu: An electron paramagnetic resonance and gamma spectroscopy study

    SciTech Connect

    Recker, M. C.; McClory, J. W. Holston, M. S.; Golden, E. M.; Giles, N. C.; Halliburton, L. E.

    2014-06-28

    Transmutation of {sup 64}Zn to {sup 65}Cu has been observed in a ZnO crystal irradiated with neutrons. The crystal was characterized with electron paramagnetic resonance (EPR) before and after the irradiation and with gamma spectroscopy after the irradiation. Major features in the gamma spectrum of the neutron-irradiated crystal included the primary 1115.5 keV gamma ray from the {sup 65}Zn decay and the positron annihilation peak at 511 keV. Their presence confirmed the successful transmutation of {sup 64}Zn nuclei to {sup 65}Cu. Additional direct evidence for transmutation was obtained from the EPR of Cu{sup 2+} ions (where {sup 63}Cu and {sup 65}Cu hyperfine lines are easily resolved). A spectrum from isolated Cu{sup 2+} (3d{sup 9}) ions acquired after the neutron irradiation showed only hyperfine lines from {sup 65}Cu nuclei. The absence of {sup 63}Cu lines in this Cu{sup 2+} spectrum left no doubt that the observed {sup 65}Cu signals were due to transmuted {sup 65}Cu nuclei created as a result of the neutron irradiation. Small concentrations of copper, in the form of Cu{sup +}-H complexes, were inadvertently present in our as-grown ZnO crystal. These Cu{sup +}-H complexes are not affected by the neutron irradiation, but they dissociate when a crystal is heated to 900 °C. This behavior allowed EPR to distinguish between the copper initially in the crystal and the copper subsequently produced by the neutron irradiation. In addition to transmutation, a second major effect of the neutron irradiation was the formation of zinc and oxygen vacancies by displacement. These vacancies were observed with EPR.

  20. Comprehensive {gamma}-ray spectroscopy of rotational bands in the N=Z+1 nucleus {sup 61}Zn

    SciTech Connect

    Andersson, L.-L.; Rudolph, D.; Johansson, E. K.; Andreoiu, C.; Ekman, J.; Fahlander, C.; Rietz, R. du; Ragnarsson, I.; Torres, D. A.; Carpenter, M. P.; Seweryniak, D.; Zhu, S.; Charity, R. J.; Chiara, C. J.; Hoel, C.; Reviol, W.; Sarantites, D. G.; Sobotka, L. G.; Pechenaya, O. L.

    2009-02-15

    The {sub 30}{sup 61}Zn{sub 31} nucleus has been studied via the combined data of two fusion-evaporation reaction experiments using a {sup 36}Ar beam and a {sup 28}Si target foil. The experimental setups involved the Ge array GAMMASPHERE and neutron and charged particle detectors placed around the target position. The resulting level scheme comprises about 120 excited states connected via some 180 {gamma}-ray transitions. In total, seven rotational structures were identified up to I{approx}25 or higher and compared with predictions from cranked Nilsson-Strutinsky calculations.

  1. Dual anode contact geometries for x-ray and gamma-ray spectroscopy and 3D localization

    NASA Astrophysics Data System (ADS)

    Martin, J. W.; Garson, A. B., III; Li, Q.; Lee, K.; Groza, M.; Buliga, V.; Burger, A.; Krawczynski, H.

    2009-08-01

    We report on the continued development and testing of unique types of Cadmium Zinc Telluride (CZT) detectors. Using large volume (10×20×20 mm3) CZT crystals, we contact various "dual anode" detector designs. We incorporate a segmented cathode with five regions so that the charge on all seven contacts can be used to determine the energy and the 3-D interaction location of detected X-ray and gamma-ray photons. We describe the status of the detector development program, emphasize strengths and weaknesses of the different contact configurations, and discuss possible applications of Dual Anode Detectors in radiation detection applications.

  2. A large-scale low-background liquid scintillation detector: the counting test facility at Gran Sasso

    NASA Astrophysics Data System (ADS)

    Alimonti, G.; Arpesella, C.; Bacchiocchi, G.; Balata, M.; Bellini, G.; Benziger, J.; Bonetti, S.; Brigatti, A.; Cadonati, L.; Calaprice, F. P.; Cavaletti, R.; Cecchet, G.; Chen, M.; Darnton, N.; Debari, A.; Deutsch, M.; Elisei, F.; von Feilitzsch, F.; Galbiati, C.; Garagiola, A.; Gatti, F.; Giammarchi, M. G.; Giugni, D.; Goldbrunner, T.; Golubchikov, A.; Goretti, A.; Grabar, S.; Hagner, T.; Hartmann, F.; von Hentig, R.; Heusser, G.; Ianni, A.; Jochum, J.; Johnson, M.; Laubenstein, M.; Loeser, F.; Lombardi, P.; Magni, S.; Malvezzi, S.; Manno, I.; Manuzio, G.; Masetti, F.; Mazzucato, U.; Meroni, E.; Neff, M.; Nisi, S.; Nostro, A.; Oberauer, L.; Perotti, A.; Preda, A.; Raghavan, P.; Raghavan, R. S.; Ranucci, G.; Resconi, E.; Ruscitti, P.; Scardaoni, R.; Schoenert, S.; Smirnov, O.; Tartaglia, R.; Testera, G.; Ullucci, P.; Vogelaar, R. B.; Vitale, S.; Zaimidoroga, O.

    1998-02-01

    A 4.8 m3 unsegmented liquid scintillation detector at the underground Laboratori Nazionali del Gran Sasso has shown the feasibility of multi-ton low-background detectors operating to energies as low as 250 keV. Detector construction and the handling of large volumes of liquid scintillator to minimize the background are described. The scintillator, 1.5 g PPO/L-pseudocumene, is held in a flexible nylon vessel shielded by 1000 t of purified water. The active detector volume is viewed by 100 photomultipliers, which measure time and charge for each event, from which energy, position and pulse shape are deduced. On-line purification of the scintillator by water extraction, vacuum distillation and nitrogen stripping removed radioactive impurities. Upper limits were established of < 10-7 Bq/kg-scintillator for events with energies 250 keV < E < 800 keV, and < 10-9 Bq/kg-scintillator due to the decay products of uranium and thorium. The isotopic abundance of 14C/12C in the scintillator was shown to be approximately 10-18 by extending the energy window of the detector to 25-250 keV. The 14C abundance and uranium and thorium levels in the CTF are compatible with the Borexino Solar Neutrino Experiment.

  3. Study of the Kroll-process to produce ultra-pure Ti for the low background experiments

    SciTech Connect

    Mozhevitina, Elena; Chepurnov, Alexander; Chub, Alexander; Avetissov, Igor; Glebovsky, Vadim; Nisi, Stefano; Di Vacri, Maria Laura; Suvorov, Yury

    2015-08-17

    To construct G2 & G3 low background experiments for direct Dark Matter search, a lot of ultra-pure construction materials will be needed. Our study of various Ti samples shows that the levels of contaminations of commercially available industrial Ti can varies from 0.2 to 100 mBq/kg for U/Th. It means that the metal Ti is such a promising material for future experiments if the way of production in bulk quantities with very low level of contaminations (below ∼1 mBq/kg of {sup 238}U /{sup 232}Th) would be developed. Our study of the industrial Kroll-process is focused on the possible sources of U and Th and their migration during the multistage Kroll process. To understand migration of U and Th during the Kroll process the set of other impurities available due to precise ICP-MS analysis have been studied. Preliminary results confirm that the Kroll process could be used for the ultra pure Ti sponge production while the following stages of the metal Ti production of from the Ti sponge with necessary mechanical properties need to be additionally studied.

  4. Sensitive detection of ozone by a practical resorufin-based spectroscopic probe with extremely low background signal

    PubMed Central

    Zhang, Yangyang; Shi, Wen; Li, Xiaohua; Ma, Huimin

    2013-01-01

    Ozone (O3) has attracted much attention because of its key role in human health and disease, and its detection is of great importance for various biochemical studies as well as environmental evaluation. Here we develop a simple and practical spectroscopic off-on O3 probe based on resorufin and the specific reaction of but-3-enyl with O3. The probe shows an extremely low background spectroscopic signal, but reacts with O3 producing a distinct color and fluorescence change. The detection limit of the probe for O3 is 5.9 nM, which corresponds to an ozone concentration of 0.056 mg m−3 in air in this study and is lower than the international ambient air quality standard of 0.1 mg m−3. More importantly, the proposed probe is worth popularizing, and its applicability has been successfully demonstrated on both the determination of O3 in real ambient air samples and the imaging of O3 in biological cells. PMID:24088783

  5. A generalized method for characterization of 235U and 239Pu content using short-lived fission product gamma spectroscopy

    DOE PAGESBeta

    Knowles, Justin R.; Skutnik, Steven E.; Glasgow, David C.; Kapsimalis, Roger J.

    2016-06-23

    Rapid non-destructive assay methods for trace fissile material analysis are needed in both nuclear forensics and safeguards communities. To address these needs, research at the High Flux Isotope Reactor Neutron Activation Analysis laboratory has developed a generalized non-destructive assay method to characterize materials containing fissile isotopes. This method relies on gamma-ray emissions from short-lived fission products and capitalizes off of differences in fission product yields to identify fissile compositions of trace material samples. Although prior work has explored the use of short-lived fission product gamma-ray measurements, the proposed method is the first to provide a holistic characterization of isotopic identification,more » mass ratios, and absolute mass determination. Successful single fissile isotope mass recoveries of less than 6% error have been conducted on standards of 235U and 239Pu as low as 12 nanograms in less than 10 minutes. Additionally, mixtures of fissile isotope standards containing 235U and 239Pu have been characterized as low as 229 nanograms of fissile mass with less than 12% error. The generalizability of this method is illustrated by evaluating different fissile isotopes, mixtures of fissile isotopes, and two different irradiation positions in the reactor. Furthermore, it is anticipated that this method will be expanded to characterize additional fissile nuclides, utilize various irradiation sources, and account for increasingly complex sample matrices.« less

  6. A GENERALIZED METHOD FOR CHARACTERIZATION OF 235U AND 239PU CONTENT USING SHORT-LIVED FISSION PRODUCT GAMMA SPECTROSCOPY

    SciTech Connect

    Knowles, Justin R; Skutnik, Steven E; Glasgow, David C; Kapsimalis, Roger J

    2016-01-01

    Rapid non-destructive assay methods for trace fissile material analysis are needed in both nuclear forensics and safeguards communities. To address these needs, research at the High Flux Isotope Reactor Neutron Activation Analysis laboratory has developed a generalized non-destructive assay method to characterize materials containing fissile isotopes. This method relies on gamma-ray emissions from short-lived fission products and capitalizes off of differences in fission product yields to identify fissile compositions of trace material samples. Although prior work has explored the use of short-lived fission product gamma-ray measurements, the proposed method is the first to provide a holistic characterization of isotopic identification, mass ratios, and absolute mass determination. Successful single fissile isotope mass recoveries of less than 6% error have been conducted on standards of 235U and 239Pu as low as 12 nanograms in less than 10 minutes. Additionally, mixtures of fissile isotope standards containing 235U and 239Pu have been characterized as low as 229 nanograms of fissile mass with less than 12% error. The generalizability of this method is illustrated by evaluating different fissile isotopes, mixtures of fissile isotopes, and two different irradiation positions in the reactor. It is anticipated that this method will be expanded to characterize additional fissile nuclides, utilize various irradiation sources, and account for increasingly complex sample matrices.

  7. Gamma-ray spectrometry of LDEF samples

    SciTech Connect

    Winn, W.G.

    1991-01-01

    A total of 31 samples from the Long Duration Exposure Facility (LDEF), including materials of aluminum, vanadium, and steel trunnions were analyzed by ultra-low-level gamma spectroscopy. The study quantified particle induced activations of (sup 22)Na, {sup 46}Sc, {sup 51}Cr, {sup 54}Mn, {sup 56}Co, {sup 57}Co, {sup 58}Co, and {sup 60}Co. The samples of trunnion sections exhibited increasing activity toward the outer end of the trunnion and decreasing activity toward its radial center. The trunnion sections did not include end pieces, which have been reported to collect noticeable {sup 7}Be on their leading surfaces. No significant {sup 7}Be was detected in the samples analyzed. The Underground Counting Facility at Savannah River Laboratory (SRL) was used in this work. The facility is 50 ft. underground, constructed with low-background shielding materials, and operated as a clean room. The most sensitive analyses were performed with a 90%-efficient HPGe gamma-ray detector, which is enclosed in a purged active/passive shield. Each sample was counted for one to six days in two orientations to yield more representative average activities for the sample. The non-standard geometries of the LDEF samples prompted the development of a novel calibration method, whereby the efficiency about the samples surfaces (measured with point sources) predicted the efficiency for the bulk sample.

  8. A study of reversible gamma-induced structural transformations in vitreous Ge23.5Sb11.8S64.7 by high-resolution X-ray photoelectron spectroscopy.

    PubMed

    Kovalskiy, Andriy; Jain, Himanshu; Miller, Alfred C; Golovchak, Roman Ya; Shpotyuk, Oleh I

    2006-11-16

    The structural origin of reversible gamma-induced effects in vitreous Ge(23.5)Sb(11.8)S(64.7) has been investigated by high-resolution X-ray photoelectron spectroscopy (XPS). The changes in valence band spectrum from gamma-irradiation suggest a decrease of sulfur lone pair electron concentration accompanied by changes in bonding states of S and Ge. The appearance of additional doublets in the core-level XPS spectra of Ge, Sb, and S atoms for gamma-irradiated sample is described by the formation of over- and under-coordinated charged defect pairs (Ge(3)(-)-S(3)(+)) as a result of radiation treatment. The results verify the switching of Ge-S covalent bonds into S-S bonds as the main microstructural mechanism for gamma-induced optical effects in this glass. PMID:17092046

  9. Cross-Section Measurements for (n,xn) Reactions by In-Beam Gamma-Ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    Pavlik, A.; Baumann, P.; Borcea, C.; Jericha, E.; Jokić, S.; Kerveno, M.; Lukić, S.; Meulders, J. P.; Mihailescu, L. C.; Nolte, R.; Plompen, A. J. M.; Raškinytė, I.; N Tof Collaboration

    2005-05-01

    The nuclear reactions 207Pb(n,2n)206Pb and 232Th(n,5n)228Th were studied by measuring prompt gamma-ray emission spectra from the interaction of neutrons with an enriched 207Pb sample and a natTh sample. For 207Pb the measurements were performed at the white neutron beam of the GELINA neutron source at IRMM Geel in the neutron energy range up to 20 MeV. The Th measurements were done at the quasi-monoenergetic 7Li(p,n)7Be neutron source at the Université Catholique de Louvain for five peak neutron energies in the range 29 MeV to 42 MeV. The measurements were complemented by model calculations using the code system EMPIRE-II.

  10. Study of heavy element structure with in-beam. cap alpha. /sup -/,. beta. /sup -/ and. gamma. -ray spectroscopy

    SciTech Connect

    Meyer, R.A.; Decman, D.J.; Henry, E.A.; Hoff, R.W.; Mann, L.G.; Struble, G.L.; Ussery, L.E.

    1984-05-10

    We describe our in-beam superconducting conversion electron spectrometer and its use in a (t,p) proton-conversion electron coincidence mode. Several examples of completed and on-going investigations are presented. These include: E0 strength from the /sup 238/U fission isomer; electromagnetic properties of the J/sup ..pi../ = 6/sup +/ and 8/sup +/ states of /sup 210/Pb; single particle and cluster states of /sup 213/Fr; the J/sup ..pi../ = 21/2/sup +/ isomer in /sup 197/Au and /sup 199/Au; and the cluster states of /sup 199/Au. Results of the study of odd-odd deformed /sup 244/Am are presented. The latter results performed using neutron-capture gamma-ray and conversion electron techniques are compared to recent developments in the modeling of deformed odd-odd nuclei. 23 refs., 10 figs., 1 tab.

  11. Characterization and identification of gamma-irradiated sauces by electron spin resonance spectroscopy using different sample pretreatments.

    PubMed

    Akram, Kashif; Ahn, Jae-Jun; Kwon, Joong-Ho

    2013-06-01

    Tomato ketchup, barbeque sauce, sweet chili sauce, and spaghetti sauce were gamma irradiated at 0, 1, 5, and 10 kGy. Electron spin resonance (ESR) technique was used to characterize the irradiated sauces, targeting radiation-induced cellulose radicals and using a modified sample pretreatment method. The samples were first washed with water, and then the residues were extracted with alcohol. The non-irradiated sauces exhibited the single central signal, whose intensity showed a significant increase on irradiation. The ESR spectra from the radiation-induced cellulose radicals, with two side peaks (g=2.02012 and g=1.98516) equally spaced (± 3 mT) from the central signal, were also observed in the irradiated sauces. The improvements in the central (natural) and radiation-induced (two side peaks corresponding to the cellulose radicals) signal intensities were obvious, when compared with routine freeze-drying and alcoholic-extraction techniques. PMID:23411320

  12. Cross-Section Measurements for (n,xn) Reactions by In-Beam Gamma-Ray Spectroscopy

    SciTech Connect

    Pavlik, A.; Baumann, P.; Kerveno, M.; Rudolf, G.; Borcea, C.; Mihailescu, L.C.; Jericha, E.; Raskinyte, I.; Jokic, S.; Lukic, S.; Meulders, J.P.; Nolte, R.; Plompen, A.J.M.

    2005-05-24

    The nuclear reactions 207Pb(n,2n)206Pb and 232Th(n,5n)228Th were studied by measuring prompt gamma-ray emission spectra from the interaction of neutrons with an enriched 207Pb sample and a natTh sample. For 207Pb the measurements were performed at the white neutron beam of the GELINA neutron source at IRMM Geel in the neutron energy range up to 20 MeV. The Th measurements were done at the quasi-monoenergetic 7Li(p,n)7Be neutron source at the Universite Catholique de Louvain for five peak neutron energies in the range 29 MeV to 42 MeV. The measurements were complemented by model calculations using the code system EMPIRE-II.

  13. FIRST-YEAR RESULTS OF BROADBAND SPECTROSCOPY OF THE BRIGHTEST FERMI-GBM GAMMA-RAY BURSTS

    SciTech Connect

    Bissaldi, Elisabetta; Von Kienlin, Andreas; Greiner, Jochen; Gruber, David; Lichti, Giselher; Diehl, Roland; Foley, Suzanne; Kouveliotou, Chryssa; Fishman, Gerald J.; Fitzpatrick, Gerard; Gibby, Melissa H.; Giles, Misty M.; Van der Horst, Alexander J.

    2011-06-01

    We present our results of the temporal and spectral analysis of a sample of 52 bright and hard gamma-ray bursts (GRBs) observed with the Fermi Gamma-ray Burst Monitor (GBM) during its first year of operation (2008 July-2009 July).Our sample was selected from a total of 253 GBM GRBs based on the event peak count rate measured between 0.2 and 40 MeV. The final sample comprised of 34 long and 18 short GRBs. These numbers show that the GBM sample contains a much larger fraction of short GRBs than the CGRO/BATSE data set, which we explain as the result of our (different) selection criteria, which favor collection of short, bright GRBs over BATSE. A first by-product of our selection methodology is the determination of a detection threshold from the GBM data alone, above which GRBs most likely will be detected in the MeV/GeV range with the Large Area Telescope on board Fermi. This predictor will be very useful for future multi-wavelength GRB follow-ups with ground- and space-based observatories. Further, we have estimated the burst durations up to 10 MeV and for the first time expanded the duration-energy relationship in the GRB light curves to high energies. We confirm that GRB durations decline with energy as a power law with index approximately -0.4, as was found earlier with the BATSE data and we also notice evidence of a possible cutoff or break at higher energies. Finally, we performed time-integrated spectral analysis of all 52 bursts and compared their spectral parameters with those obtained with the larger data sample of the BATSE data. We find that the two parameter data sets are similar and confirm that short GRBs are in general harder than longer ones.

  14. First-year Results of Broadband Spectroscopy of the Brightest Fermi-GBM Gamma-Ray Bursts

    NASA Astrophysics Data System (ADS)

    Bissaldi, Elisabetta; von Kienlin, Andreas; Kouveliotou, Chryssa; Briggs, Michael S.; Connaughton, Valerie; Greiner, Jochen; Gruber, David; Lichti, Giselher; Bhat, P. N.; Burgess, Michael; Chaplin, Vandiver; Diehl, Roland; Fishman, Gerald J.; Fitzpatrick, Gerard; Foley, Suzanne; Gibby, Melissa H.; Giles, Misty M.; Goldstein, Adam; Guiriec, Sylvain; van der Horst, Alexander J.; Kippen, R. Marc; Lin, Lin; McBreen, Sheila; Meegan, Charles A.; Paciesas, William S.; Preece, Robert D.; Rau, Arne; Tierney, Dave; Wilson-Hodge, Colleen

    2011-06-01

    We present our results of the temporal and spectral analysis of a sample of 52 bright and hard gamma-ray bursts (GRBs) observed with the Fermi Gamma-ray Burst Monitor (GBM) during its first year of operation (2008 July-2009 July).Our sample was selected from a total of 253 GBM GRBs based on the event peak count rate measured between 0.2 and 40 MeV. The final sample comprised of 34 long and 18 short GRBs. These numbers show that the GBM sample contains a much larger fraction of short GRBs than the CGRO/BATSE data set, which we explain as the result of our (different) selection criteria, which favor collection of short, bright GRBs over BATSE. A first by-product of our selection methodology is the determination of a detection threshold from the GBM data alone, above which GRBs most likely will be detected in the MeV/GeV range with the Large Area Telescope on board Fermi. This predictor will be very useful for future multi-wavelength GRB follow-ups with ground- and space-based observatories. Further, we have estimated the burst durations up to 10 MeV and for the first time expanded the duration-energy relationship in the GRB light curves to high energies. We confirm that GRB durations decline with energy as a power law with index approximately -0.4, as was found earlier with the BATSE data and we also notice evidence of a possible cutoff or break at higher energies. Finally, we performed time-integrated spectral analysis of all 52 bursts and compared their spectral parameters with those obtained with the larger data sample of the BATSE data. We find that the two parameter data sets are similar and confirm that short GRBs are in general harder than longer ones.

  15. Search for 2{nu}{beta}{beta} Decay of {sup 130}Te to the First Excited State of {sup 130}Xe with an Ultra-Low-Background Germanium Crystal Array

    SciTech Connect

    Mizouni, L. K.; Aalseth, C. E.; Erikson, L. E.; Hossbach, T. W.; Keillor, M. E.; Orrell, J. L.; Avignone, F. T. III

    2011-12-13

    The goal of searching for zero-neutrino double-beta (0{nu}{beta}{beta}) decay is to probe an absolute neutrino mass scale suggested by the mass-splitting parameters observed by neutrino oscillation experiments. Furthermore, observation of 0{nu}{beta}{beta} decay is an explicit instance of Lepton-number non-conservation. A sensitive measurement of two-neutrino double-beta (2{nu}{beta}{beta}) decay can provide critical input to Quasiparticle Random Phase Approximation (QRPA) calculations of the nuclear matrix elements in models similar to those used to extract the absolute neutrino mass from (0{nu}{beta}{beta}) decay experiments. Tellurium-130, an even-even nucleus, can undergo 2{nu}{beta}{beta} decay to the first 0+ excited state of {sup 130}Xe producing three possible {gamma}-ray cascades as it transitions to the ground state. The Cascades detector is a high purity germanium (HPGe) crystal array consisting of two ultra-low-background copper cryostats each housing a hexagonal array of seven crystals. The project is currently being developed at Pacific Northwest National Laboratory in Richland, WA (USA), and aims to obtain very high {gamma}-ray detection efficiency while utilizing highly effective and low-background shielding. GEANT4 simulations of the detector are performed for a {sup 130}Te sample in order to determine the optimum size and geometry of the source for maximum detection efficiency and predict its sensitivity for measuring 2{nu}{beta}{beta} decay to the first 0+ excited state of {sup 130}Xe. These simulations are validated with calibration sources and presented.

  16. LOW-RESOLUTION SPECTROSCOPY OF GAMMA-RAY BURST OPTICAL AFTERGLOWS: BIASES IN THE SWIFT SAMPLE AND CHARACTERIZATION OF THE ABSORBERS

    SciTech Connect

    Fynbo, J. P. U.; Malesani, D.; Vreeswijk, P. M.; Hjorth, J.; Sollerman, J.; Thoene, C. C.; Jakobsson, P.; Bjoernsson, G.; De Cia, A.; Prochaska, J. X.; Nardini, M.; Chen, H.-W.; Bloom, J. S.; Castro-Tirado, A. J.; Gorosabel, J.; Christensen, L.; Fruchter, A. S.

    2009-12-01

    We present a sample of 77 optical afterglows (OAs) of Swift detected gamma-ray bursts (GRBs) for which spectroscopic follow-up observations have been secured. Our first objective is to measure the redshifts of the bursts. For the majority (90%) of the afterglows, the redshifts have been determined from the spectra. We provide line lists and equivalent widths (EWs) for all detected lines redward of Ly{alpha} covered by the spectra. In addition to the GRB absorption systems, these lists include line strengths for a total of 33 intervening absorption systems. We discuss to what extent the current sample of Swift bursts with OA spectroscopy is a biased subsample of all Swift detected GRBs. For that purpose we define an X-ray-selected statistical sample of Swift bursts with optimal conditions for ground-based follow-up from the period 2005 March to 2008 September; 146 bursts fulfill our sample criteria. We derive the redshift distribution for the statistical (X-ray selected) sample and conclude that less than 18% of Swift bursts can be at z > 7. We compare the high-energy properties (e.g., {gamma}-ray (15-350 keV) fluence and duration, X-ray flux, and excess absorption) for three subsamples of bursts in the statistical sample: (1) bursts with redshifts measured from OA spectroscopy; (2) bursts with detected optical and/or near-IR afterglow, but no afterglow-based redshift; and (3) bursts with no detection of the OA. The bursts in group (1) have slightly higher {gamma}-ray fluences and higher X-ray fluxes and significantly less excess X-ray absorption than bursts in the other two groups. In addition, the fractions of dark bursts, defined as bursts with an optical to X-ray slope {beta}{sub OX} < 0.5, is 14% in group (1), 38% in group (2), and >39% in group (3). For the full sample, the dark burst fraction is constrained to be in the range 25%-42%. From this we conclude that the sample of GRBs with OA spectroscopy is not representative for all Swift bursts, most likely due

  17. Fully automated radiochemical preparation system for gamma-spectroscopy on fission products and the study of the intruder and vibrational levels in /sup 83/Se

    SciTech Connect

    Lien, O.G. III

    1983-10-01

    AUTOBATCH was developed to provide a usable source of short-lived neutron-rich nuclides through chemical preparation of the sample from fission products for detailed gamma-ray spectroscopy, which would complement the output of on-line isotope separators. With AUTOBATCH the gamma rays following the ..beta../sup -/ decay of /sup 83/As were studied to determine the ground state spin and parity of /sup 83/As to be 5/2/sup -/; the absolute intensity of the ..beta../sup -/ branch from /sup 83/As to /sup 83/Se/sup m/ to be 0.3%; the absolute intensity of the ground state ..beta../sup -/ branch from /sup 83/Se/sup m/ to /sup 83/Br to be 39%; the halflife of the 5/2/sub 1//sup +/ level to be 3.2 ns; and the structure of /sup 83/Se/sub 49/. Results are used to show that the intruder structure which had been previously observed in the odd mass /sub 49/In isotopes could be observed in the N = 49 isotones. The observed structure is discussed in terms of the unified model calculations of Heyde which has been used to describe the intruder structure in the indium nuclei. The intruder structure is most strongly developed, not at core mid-shell, /sup 89/Zr/sub 49/, but rather at core mid-sub-shell /sup 83/Se. This difference is qualitatively understood to be due to the blocking of collectivity by the Z = 40 subshell closure which prevents the intruder structure from occurring in /sup 87/Sr/sub 49/ and /sup 89/Zr/sub 49/.

  18. Development of the Experimental Setup Dedicated for Alpha, Gamma and Electron Spectroscopy of Heavy Nuclei at FLNR JINR

    SciTech Connect

    Yeremin, A.; Malyshev, O.; Popeko, A.; Lopez-Martens, A.; Hauschild, K.; Dorvaux, O.; Saro, S.; Pantelika, D.

    2010-04-30

    Various types of reactions and identification techniques were applied in the investigation of formation cross sections and decay properties of transuranium elements. The fusion--evaporation reactions with heavy targets, recoil--separation techniques and identification of nuclei by the parent--daughter generic coincidences with the known daughter-nuclei after implantation into position--sensitive detectors were the most successful tools for production and identification of the heaviest elements known presently. This technique may be further improved and presently it may be very promising for the identification of new elements, search for new isotopes and measurement of new decay data for the known nuclei.At the Flerov Laboratory of Nuclear Reactions (JINR, Dubna), investigations of the complete fusion reactions leading to the synthesis of heavy and superheavy nuclei with the use of heavy ion beams from a powerful U400 cyclotron have been an important part of the experimental program. It is planned to upgrade U400 cyclotron of the FLNR, to deliver beams with higher intensities and smooth variation of energies.New experimental set up, the velocity filter, is now developing for synthesis and studies of the decay properties of heavy nuclei. At the focal plane of the separator GABRIELA set up (alpha,beta,gamma detectors array) will be installed.

  19. Interpretations and implications of gamma ray lines from solar flares, the galactic center in gamma ray transients

    NASA Technical Reports Server (NTRS)

    Ramaty, R.; Lingenfelter, R. E.

    1980-01-01

    Observations and theories of astrophysical gamma ray line emission are reviewed and prospects for future observations by the spectroscopy experiments on the planned Gamma Ray Observatory are discussed.

  20. Application of high resolution NMR, ESR, and gamma-ray scintillation spectroscopy to the study of ligand binding in proteins. [Torpedo californica

    SciTech Connect

    Lancione, G.V.

    1982-01-01

    Electron spin resonance spectroscopy has been employed to study the nature of the ligand binding site of alpha-1-antitrypsin. Spectra of spin-labeled alpha-1-antitrypsin were recorded at pH's ranging from 2.4 to 12.5. This data demonstrates the tight binding of the spin-label to the protease, and the sensitivity of the bound spin-label to informational changes in the protease inhibitor. A molecular dipstick approach has also been applied to this system and has yielded information on the geometry of the cleft accommodating the spin-label. /sup 160/Terbium(III) exchange experiments have been performed on the acetylcholine receptor protein isolated from Torpedo californica, employing a specially designed flow dialysis apparatus constructed in the laboratory. The apparatus is designed to allow continuous monitoring of /sup 160/Tb(III) gamma-ray emission from the protein compartment of the flow dialysis cell. Nicotinic ligand-induced displacement of /sup 160/Tb(III) from the nicotinic binding site of the receptor was monitored as a funtion of (1) the concentration of nicotinic ligand in the washout buffer, and (2) the nature of the nicotinic ligand in the buffer. Measured /sup 160/Tb(III) exchange half-lives indicate (1) a direct relationship between /sup 160/Tb(III) displacement and nicotinic ligand concentration in the wash-out buffer, and (2) an enhanced /sup 160/Tb(III) displacement for nicotinic agents possessing quaternary ammonium functions.

  1. Extending the Astronomical Application of Photon Counting HgCdTe Linear Avalanche Photo-Diode Arrays to Low Background Space Observations.

    NASA Astrophysics Data System (ADS)

    Hall, Donald

    infrared photon counting performance at the low and ultra-low backgrounds required for NASA space astronomy missions. Specifically this will involve 1) Measuring the gain normalized dark count rate and avalanche gain of 2.5, 3.3 and 4 micron cutoff HgCdTe at cryogenic temperatures from 30 to 80 K and bias voltages up to 20 V, 2) Using these results to validate and refine models of avalanche gain along with generation- recombination and surface trap induced tunneling current in L-APD HgCdTe and, 3) Modeling the gain normalized dark count rate, surface tunneling current and avalanche gain of 2 to 5 micron cutoff HgCdTe L-APD arrays for astrophysics and other NASA missions. The overall objective of the investigation is to develop the tools to identify the sweet spot in bandgap and cryogenic operating temperature for each specific NASA astrophysics mission and to accurately predict ultimate performance. HgCdTe L-APD technology offers to NASA the ultimate performance for space astronomy in photon starved applications such as: 1) ultra-low background, extra- Zodiacal imaging and faint object spectroscopy from elliptical orbits beyond the asteroid belt with missions such as Extra-Zodiacal Explorer, 2) spectroscopy of the faintest O/IR sources from near earth and L-2 orbit at moderate to high resolution and, 3) time domain astronomy observations (photometric or spectral variations at frequencies above 1 Hz) of sources as diverse as close binaries, accretion disks, compact objects etc. HgCdTe L- APD arrays have the potential to enable new classes of missions and to bring critical observations within reach of the capabilities of the NASA SMD Astrophysics Explorer program. As they utilize the same mature TRL base as the large format JWST HgCdTe arrays, requiring only qualification of n-on-p material operated at higher bias voltages, the path to flight qualification is unusually direct.

  2. RESEARCH NOTE FROM COLLABORATION: Production and decay of the 73Ge*(1/2-) metastable state in a low-background germanium detector

    NASA Astrophysics Data System (ADS)

    Liao, H. Y.; Chang, H. M.; Chou, M. H.; Deniz, M.; Huang, H. X.; Lee, F. S.; Li, H. B.; Li, J.; Lin, C. W.; Lin, F. K.; Lin, S. K.; Lin, S. T.; Singh, V.; Wong, H. T.; Wu, S. C.; TEXONO Collaboration

    2008-07-01

    The 73Ge*(1/2-) metastable state decays with a very characteristic signature which allows it to be tagged event-by-event. Studies were performed using data taken with a high-purity germanium detector in a low-background laboratory near a nuclear power reactor core where the \\rm{\\bar{\

  3. Nano {gamma}'/{gamma}'' composite precipitates in Alloy 718

    SciTech Connect

    Phillips, P. J.; McAllister, D.; Gao, Y.; Lv, D.; Williams, R. E. A.; Wang, Y.; Mills, M. J.; Peterson, B.

    2012-05-21

    Nanoscale composite precipitates of Alloy 718 have been investigated with both high-resolution scanning transmission electron microscopy and phase field modeling. Chemical analysis via energy-dispersive x-ray spectroscopy allowed for the differentiation of {gamma}' and {gamma}'' particles, which is not otherwise possible through traditional Z-contrast methods. Phase field modeling was applied to determine the stress distribution and elastic interaction around and between the particles, respectively, and it was determined that a composite particle (of both {gamma}' and {gamma}'') has an elastic energy that is significantly lower than, for example, single {gamma}' and {gamma}'' precipitates which are non-interacting.

  4. SYNTH - Gamma Ray Spectrum Synthesizer

    Energy Science and Technology Software Center (ESTSC)

    2009-05-18

    SYNTH was designed to synthesize the results of typical gamma-ray spectroscopy experiments. The code allows a user to specify the physical characteristics of a gamma-ray source, the quantity of radionuclides emitting gamma radiation, the source-to-detector distance and the presence and type of any intervening absorbers, the size and type of the gamma-ray detector, and the electronic set-up used to gather the data.

  5. To Sample or Not to Sample - An Investigation Into the Uncertainty from Sampling Followed by Laboratory Analysis Versus In-Toto Gamma Spectroscopy for Situations of Non-Uniform Radioactivity Distribution

    SciTech Connect

    Bronson, F.

    2008-07-01

    During the decommissioning of structures and the remediation of soil, material that is known or suspected to be contaminated with radioactivity must be assayed. For many, if not most, of the cases, the radioactive material concentration can be determined or inferred by gamma spectroscopy. In most, if not all, of these cases, the radioactivity is not uniformly distributed. For these situations, is it better to perform in-toto measurements of the entire item, or is it better to extract a sample and analyze that sample? For the in-toto gamma spectroscopy measurement, the results will not be accurate unless the calibration method perfectly represents the measured item. And since the calibrations normally assume uniformly distributed radioactivity, any nonuniform distribution of radioactivity in the measured material will cause an error in the results. A mathematical program using probabilistic methods has been developed to estimate the uncertainty in in-toto gamma spectroscopy measurements. This program has the capability of determining the efficiency of various types of non-uniform radioactivity distributions and to compare it to the uniform distribution efficiency. Repeating this for a large number of random tries allows the estimation of the measurement uncertainty. A new feature has been added to the program to simulate the extraction of a sample from these same non-uniform distributions, to compute the average concentration in this extracted sample, and to compare it to the average concentration in the original item to be measured. Repeating this for a large number of random tries allows the estimation of the sampling uncertainty. These two computations were run on several different 'typical' contamination measurement scenarios [200 liter drums, 27 cubic meter 'truck' containers, 0.01-10 liter 'laboratory' containers, and 3600 square meter soil 'in-situ' plots]. In all cases examined, the sampling uncertainty was larger than the in-toto gamma measurement

  6. Gamma ray spectrometry of LDEF samples at SRL

    NASA Astrophysics Data System (ADS)

    Winn, W. G.

    1991-07-01

    A total of 31 samples from the Long Duration Exposure Facility (LDEF), including materials of aluminum, vanadium, and steel trunnions were analyzed by ultra-low-level gamma spectroscopy. The study quantified particle induced activations of Na-22, Sc-46, Cr-51, Mn-54, Co-56, Co-57, Co-58, and Co-60. The samples of trunnion sections exhibited increasing activity toward the outer end of the trunnion and decreasing activity toward its radial center. The trunnion sections did not include end pieces, which have been reported to collect noticeable Be-7 on their leading surfaces. No significant Be-7 was detected in the samples analyzed. The Underground Counting Facility at Savannah River Laboratory (SRL) was used in this work. The facility is 50 ft. underground, constructed with low-background shielding materials, and operated as a clean room. The most sensitive analyses were performed with a 90 percent efficient HPGe gamma-ray detector, which is enclosed in a purged active/passive shield. Each sample was counted for one to six days in two orientations to yield more representative average activities for the sample. The non-standard geometries of the LDEF samples prompted the development of a novel calibration method, whereby the efficiency about the samples surfaces (measured with point sources) predicted the efficiency for the bulk sample.

  7. Resonance production in. gamma gamma. collisions

    SciTech Connect

    Renard, F.M.

    1983-04-01

    The processes ..gamma gamma.. ..-->.. hadrons can be depicted as follows. One photon creates a q anti q pair which starts to evolve; the other photon can either (A) make its own q anti q pair and the (q anti q q anti q) system continue to evolve or (B) interact with the quarks of the first pair and lead to a modified (q anti q) system in interaction with C = +1 quantum numbers. A review of the recent theoretical activity concerning resonance production and related problems is given under the following headings: hadronic C = +1 spectroscopy (q anti q, qq anti q anti q, q anti q g, gg, ggg bound states and mixing effects); exclusive ..gamma gamma.. processes (generalities, unitarized Born method, VDM and QCD); total cross section (soft and hard contributions); q/sup 2/ dependence of soft processes (soft/hard separation, 1/sup +- +/ resonances); and polarization effects. (WHK)

  8. A Team Approach to the Development of Gamma Ray and x Ray Remote Sensing and in Situ Spectroscopy for Planetary Exploration Missions

    NASA Technical Reports Server (NTRS)

    Trombka, J. I.; Floyd, S.; Ruitberg, A.; Evans, L.; Starr, R.; Metzger, A.; Reedy, R.; Drake, D.; Moss, C.; Edwards, B.

    1993-01-01

    An important part of the investigation of planetary origin and evolution is the determination of the surface composition of planets, comets, and asteroids. Measurements of discrete line X-ray and gamma ray emissions from condensed bodies in space can be used to obtain both qualitative and quantitative elemental composition information. The Planetary Instrumentation Definition and Development Program (PIDDP) X-Ray/Gamma Ray Team has been established to develop remote sensing and in situ technologies for future planetary exploration missions.

  9. Peak shifted properties of the "low background NaI(Tl) detectors": An experimental study of response function behavior in different temperature and acquisition time

    NASA Astrophysics Data System (ADS)

    Rezaei Moghaddam, Y.; Rafat Motavalli, L.; Miri Hakimabadi, H.

    2016-09-01

    Due to the necessity of using low background NaI detector in sensitive and accurate measurements, study on the response function variations in different conditions is very important. These types of detectors have different responses in various measurement conditions, including time, temperature and high voltage. In this study, the response function of 76 B 76 LB NaI (SCIONIX) in different conditions is discussed. According to the channel shifting in these detectors and its direct effect on degrading the resolution, the most convenient measurement condition for these detectors, is proposed. Finally, it is recommended that before long-time measurements a "waiting time" is needed to avoid the channel shifting effects.

  10. Low background techniques in CANDLES

    NASA Astrophysics Data System (ADS)

    Nakajima, K.; Iida, T.; Kishimoto, T.; Matsuoka, K.; Nomachi, M.; Umehara, S.; Chan, W. M.; Kakubata, H.; Li, X.; Maeda, T.; Ohata, T.; Temuge, B.; Tetsuno, K.; Trang, V. T. T.; Uehara, T.; Yoshida, S.; Morishita, K.; Ogawa, I.; Sakamoto, K.; Tamagawa, Y.; Yoshizawa, M.; Fushimi, K.; Hazama, R.; Naktani, N.; Suzuki, K.

    2015-08-01

    CANDLES is a double beta decay experiment using 48Ca in CaF2 crystals. The measurement is being performed with prototype detector (CANDLES III) for high sensitive measurement in the future. Recent status of detector improvements and background reduction techniques are described in this paper.

  11. Low background techniques in CANDLES

    SciTech Connect

    Nakajima, K. E-mail: nkyohei@u-fukui.ac.jp; Iida, T.; Matsuoka, K.; Nomachi, M.; Umehara, S.; Kishimoto, T.; Chan, W. M.; Kakubata, H.; Li, X.; Maeda, T.; Ohata, T.; Temuge, B.; Tetsuno, K.; Trang, V. T. T.; Uehara, T.; Yoshida, S.; Morishita, K.; Ogawa, I.; Sakamoto, K.; Tamagawa, Y.; and others

    2015-08-17

    CANDLES is a double beta decay experiment using {sup 48}Ca in CaF{sub 2} crystals. The measurement is being performed with prototype detector (CANDLES III) for high sensitive measurement in the future. Recent status of detector improvements and background reduction techniques are described in this paper.

  12. Low-resolution Spectroscopy of Gamma-ray Burst Optical Afterglows: Biases in the Swift Sample and Characterization of the Absorbers

    NASA Astrophysics Data System (ADS)

    Fynbo, J. P. U.; Jakobsson, P.; Prochaska, J. X.; Malesani, D.; Ledoux, C.; de Ugarte Postigo, A.; Nardini, M.; Vreeswijk, P. M.; Wiersema, K.; Hjorth, J.; Sollerman, J.; Chen, H.-W.; Thöne, C. C.; Björnsson, G.; Bloom, J. S.; Castro-Tirado, A. J.; Christensen, L.; De Cia, A.; Fruchter, A. S.; Gorosabel, J.; Graham, J. F.; Jaunsen, A. O.; Jensen, B. L.; Kann, D. A.; Kouveliotou, C.; Levan, A. J.; Maund, J.; Masetti, N.; Milvang-Jensen, B.; Palazzi, E.; Perley, D. A.; Pian, E.; Rol, E.; Schady, P.; Starling, R. L. C.; Tanvir, N. R.; Watson, D. J.; Xu, D.; Augusteijn, T.; Grundahl, F.; Telting, J.; Quirion, P.-O.

    2009-12-01

    We present a sample of 77 optical afterglows (OAs) of Swift detected gamma-ray bursts (GRBs) for which spectroscopic follow-up observations have been secured. Our first objective is to measure the redshifts of the bursts. For the majority (90%) of the afterglows, the redshifts have been determined from the spectra. We provide line lists and equivalent widths (EWs) for all detected lines redward of Lyα covered by the spectra. In addition to the GRB absorption systems, these lists include line strengths for a total of 33 intervening absorption systems. We discuss to what extent the current sample of Swift bursts with OA spectroscopy is a biased subsample of all Swift detected GRBs. For that purpose we define an X-ray-selected statistical sample of Swift bursts with optimal conditions for ground-based follow-up from the period 2005 March to 2008 September; 146 bursts fulfill our sample criteria. We derive the redshift distribution for the statistical (X-ray selected) sample and conclude that less than 18% of Swift bursts can be at z > 7. We compare the high-energy properties (e.g., γ-ray (15-350 keV) fluence and duration, X-ray flux, and excess absorption) for three subsamples of bursts in the statistical sample: (1) bursts with redshifts measured from OA spectroscopy; (2) bursts with detected optical and/or near-IR afterglow, but no afterglow-based redshift; and (3) bursts with no detection of the OA. The bursts in group (1) have slightly higher γ-ray fluences and higher X-ray fluxes and significantly less excess X-ray absorption than bursts in the other two groups. In addition, the fractions of dark bursts, defined as bursts with an optical to X-ray slope βOX < 0.5, is 14% in group (1), 38% in group (2), and >39% in group (3). For the full sample, the dark burst fraction is constrained to be in the range 25%-42%. From this we conclude that the sample of GRBs with OA spectroscopy is not representative for all Swift bursts, most likely due to a bias against the

  13. Gamma-Ray Pulsars

    NASA Technical Reports Server (NTRS)

    Harding, Alice K.

    2011-01-01

    The Fermi Gamma-Ray Space Telescope has revolutionized the study of pulsar physics with the detection of over 80 gamma-ray pulsars. Several new populations have been discovered, including 24 radio quiet pulsars found through gamma-ray pulsations alone and about 20 millisecond gamma-ray pulsars. The gamma-ray pulsations from millisecond pulsars were discovered by both folding at periods of known radio millisecond pulsars or by detecting them as gamma-ray sources that are followed up by radio pulsar searches. The second method has resulted in a phenomenally successful synergy, with -35 new radio MSPs (to date) having been discovered at Fermi unidentified source locations and the gamma-ray pulsations having then been detected in a number of these using the radio timing solutions. The higher sensitivity and larger energy range of the Fermi Large Area Telescope has produced detailed energy-dependent light curves and phase-resolved spectroscopy on brighter pulsars, that have ruled out polar cap models as the major source of the emission in favor of outer magnetosphere accelerators. The large number of gamma-ray pulsars now allows for the first time meaningful population and sub-population studies that are revealing surprising properties of these fascinating sources.

  14. Characterization of the (0110) {alpha}-Ti/{gamma}-TiH interface using high-resolution Transmission Electron Microscopy (TEM) and Electron Energy Loss Spectroscopy (EELS)

    SciTech Connect

    Tsai, M.M.; Howe, J.M.

    1996-12-31

    Precipitation of {gamma}-TiH in {alpha}-Ti-H alloys involves a hcp {r_arrow} fct lattice transformation with hydrogen as an interstitial diffusing element. Results obtained from a previous TEM study have shown that the lengthening rate of {gamma}-TiH is diffusionally controlled at 25{degrees}C, and possibly interfacially controlled at temperatures of 50{degrees}C and higher. Therefore, it is essential to ascertain the presence or absence of hydrogen atoms at the interface. TEM foils from a 800 ppm wt.% Ti-H alloy were analyzed using high-resolution TEM and image simulations in order to determine the effects of hydrogen on high-resolution images of the {alpha}-Ti/{gamma}-TiH interface, and EELS was used to determine the whether the hydride structure was fully formed up to the interface.

  15. Neutrons and gamma-rays spectroscopy of Mercury surface: global mapping from ESA MPO-BepiColombo spacecraft by MGNS instrument.

    NASA Astrophysics Data System (ADS)

    Kozyrev, A. S.; Gurvits, L. I.; Litvak, M. L.; Malakhov, A. A.; Mokrousov, M. I.; Mitrofanov, I. G.; Rogozhin, A. A.; Sanin, A. B.; Owens, A.; Schvetsov, V. N.

    2009-04-01

    For analyse chemistry composition of Mercury subsurface we will apply method of as-called remote sensing of neutrons. This method can be use for study celestial body of Solar system without thick atmospheres, like Moon, Mars, Phobos, Mercury etc. by the analysis of induced nuclear gamma-rays and neutron emission. These gamma-rays and neutrons are produced by energetic galactic cosmic rays colliding with nuclei of regolith within a 1-2 meter layer of subsurface. Mercury Planetary Orbiter of BepiColombo mission includes the nuclear instrument MGNS (Mercury Gamma-rays and Neutrons Spectrometers), which consists of gamma-rays spectrometer for detection of gamma-ray lines and neutron spectrometer for measurement of the neutron leakage flux. To test know theoretical models of Mercury composition, MGNS will provide the data for the set of gamma-ray lines, which are necessary and sufficient to discriminate between the models. Neutron data are known to be very sensitive for the presence of hydrogen within heavy soil-constituting elements. Mapping measurements of epithermal neutrons and 2.2 MeV line will allow us to study the content of hydrogen over the surface of Mercury and to test the presence of water ice deposits in the cold traps of permanently shadowed polar craters of this planet. There are also three natural radioactive elements, K, Th and U, which contents in the soil of a celestial body characterizes the physical condition of its formation in the proto-planetary cloud. The data from gamma-spectrometer will allow to compare the origin of Mercury with evolution of Earth, Moon and Mars. Three sensors for thermal and epithermal neutrons are made with similar 3He proportional counters, but have different polyethylene enclosures and cadmium shielding for different sensitivity of thermal and epithermal neutrons at different energy ranges. The fourth neutron sensor for high energy neutrons 1-10 MeV contains the scintillation crystal of stylbene with cylindrical shape of

  16. Lack of Association between High-Density Lipoprotein Cholesterol and Angiographic Coronary Lesion Severity in Chinese Patients with Low Background Low-Density Lipoprotein Cholesterol

    PubMed Central

    Su, Chieh-Shou; Chen, Kuan-Ju; Sheu, Wayne Huey-Herng; Yang, Ya-Ling; Liu, Tsun-Jui; Chang, Wei-Chun; Wang, Kuo-Yang; Lee, Wen-Lieng

    2015-01-01

    Background The atheroprotective role of high-density lipoprotein (HDL-C) particles as measured by HDL-C level in coronary arterial disease (CAD) remains unsettled. The aim of our study was to ascertain whether HDL-C was associated with the development and severity of coronary artery disease in Chinese patients who underwent coronary angiogram with low background Low-density lipoprotein (LDL-C) levels, which has not been previously investigated. Methods Between March 1995 and May 2000, 566 consecutive patients (408 males, 66.7 ± 11.3 years of age) with background LDL-C less than 100 mg/dl who underwent coronary artery angiography at our cath lab for suspected CAD were retrospectively recruited into the study. The severity of coronary lesions was measured by conventional coronary angiography and modified Gensini scores. Results In those subjects with significant coronary lesions, there were more males and conventional CAD risk factors of diabetes mellitus, smoking, and chronic renal disease. They were also older compared to those in the control group. However, total cholesterol, LDL-C, HDL-C, triglyceride levels and use of statins were similar in both groups. In those subjects with significant coronary lesions, there was no difference in conventional coronary lesion severity or modified Gensini score between the quartered HDL-C subgroups. Furthermore, there was no significant correlation between serum HDL-C level and modified Gensini scores. In linear regression analysis, HDL-C was not an independent predictor for modified Gensini scores. Furthermore, HDL-C was also not an independent risk factor for the presence of significant coronary lesions in low LDL-C patients in logistic regression analysis. Conclusions In Chinese patients with low background LDL-C, serum HDL-C was not associated with development of CAD or lesion severity in patients with suspected CAD. Therefore, HDL-C did not appear to be atheroprotective in these patients. PMID:27122918

  17. Search for 2νββ Decay of 130Te to the First Excited State of 130Xe with an Ultra-Low-Background Germanium Crystal Array

    NASA Astrophysics Data System (ADS)

    Mizouni, L. K.; Aalseth, C. E.; Avignone, F. T.; Erikson, L. E.; Hossbach, T. W.; Keillor, M. E.; Orrell, J. L.

    2011-12-01

    The goal of searching for zero-neutrino double-beta (0νββ) decay is to probe an absolute neutrino mass scale suggested by the mass-splitting parameters observed by neutrino oscillation experiments. Furthermore, observation of 0νββ decay is an explicit instance of Lepton-number non-conservation. A sensitive measurement of two-neutrino double-beta (2νββ) decay can provide critical input to Quasiparticle Random Phase Approximation (QRPA) calculations of the nuclear matrix elements in models similar to those used to extract the absolute neutrino mass from (0νββ) decay experiments. Tellurium-130, an even-even nucleus, can undergo 2νββ decay to the first 0+ excited state of 130Xe producing three possible γ-ray cascades as it transitions to the ground state. The Cascades detector is a high purity germanium (HPGe) crystal array consisting of two ultra-low-background copper cryostats each housing a hexagonal array of seven crystals. The project is currently being developed at Pacific Northwest National Laboratory in Richland, WA (USA), and aims to obtain very high γ-ray detection efficiency while utilizing highly effective and low-background shielding. GEANT4 simulations of the detector are performed for a 130Te sample in order to determine the optimum size and geometry of the source for maximum detection efficiency and predict its sensitivity for measuring 2νββ decay to the first 0+ excited state of 130Xe. These simulations are validated with calibration sources and presented.

  18. Polonium–lead extractions to determine the best method for the quantification of clean lead used in low-background radiation detectors

    SciTech Connect

    Miley, Sarah M.; Payne, Rosara F.; Schulte, Shannon M.; Finn, Erin C.

    2009-12-01

    Very sensitive detectors are used for low-background applications including the detection of environmental radioactivity, double-beta decay, and dark matter. In order to reduce the background noise enough to utilize the sensitivity of these detectors, lead with little or no alpha activity is required to form the shielding. In the past, antiquity lead shielding was used for low-background detectors because lead’s most prominent alpha-emitting isotope, 210Pb, has a short half-life. The microelectronics industry is also greatly affected by alpha activity in lead and solder, and has begun producing “clean” lead for purchase. To quantify how clean the available lead is, 210Pb and, during procedural experiments, a 209Po tracer must be physically or chemically removed from the bulk lead. A reliable procedure for chemical separations that does not use large volumes of ultra-high-purity chemicals has not yet been established. Lead was dissolved and a known amount of 209Po tracer was added. The samples were put through each of two new procedures. The first procedure was based on complete dissolution of the lead followed by a column separation. The second method investigates the utility of a pre-separation step using precipitation of the lead prior to column separation. The resulting solutions were run through strontium resin columns from Eichrom Inc., a United States Transuranium and Uranium Registries (USTUR) electrodeposition procedure, and scheduled to be alpha counted for a minimum of three days. Though neither of the tested procedures had acceptable logistics for large scale implementation, later alpha counting will show which procedure is more promising for further development

  19. Assessment of individual organ doses in a realistic human phantom from neutron and gamma stimulated spectroscopy of the breast and liver

    SciTech Connect

    Belley, Matthew D.; Segars, William Paul; Kapadia, Anuj J.

    2014-06-15

    Purpose: Understanding the radiation dose to a patient is essential when considering the use of an ionizing diagnostic imaging test for clinical diagnosis and screening. Using Monte Carlo simulations, the authors estimated the three-dimensional organ-dose distribution from neutron and gamma irradiation of the male liver, female liver, and female breasts for neutron- and gamma-stimulated spectroscopic imaging. Methods: Monte Carlo simulations were developed using the Geant4 GATE application and a voxelized XCAT human phantom. A male and a female whole body XCAT phantom was voxelized into 256 × 256 × 600 voxels (3.125 × 3.125 × 3.125 mm{sup 3}). A monoenergetic rectangular beam of 5.0 MeV neutrons or 7.0 MeV photons was made incident on a 2 cm thick slice of the phantom. The beam was rotated at eight different angles around the phantom ranging from 0° to 180°. Absorbed dose was calculated for each individual organ in the body and dose volume histograms were computed to analyze the absolute and relative doses in each organ. Results: The neutron irradiations of the liver showed the highest organ dose absorption in the liver, with appreciably lower doses in other proximal organs. The dose distribution within the irradiated slice exhibited substantial attenuation with increasing depth along the beam path, attenuating to ∼15% of the maximum value at the beam exit side. The gamma irradiation of the liver imparted the highest organ dose to the stomach wall. The dose distribution from the gammas showed a region of dose buildup at the beam entrance, followed by a relatively uniform dose distribution to all of the deep tissue structures, attenuating to ∼75% of the maximum value at the beam exit side. For the breast scans, both the neutron and gamma irradiation registered maximum organ doses in the breasts, with all other organs receiving less than 1% of the breast dose. Effective doses ranged from 0.22 to 0.37 mSv for the neutron scans and 41 to 66 mSv for the gamma

  20. Assessment of individual organ doses in a realistic human phantom from neutron and gamma stimulated spectroscopy of the breast and liver

    PubMed Central

    Belley, Matthew D.; Segars, William Paul; Kapadia, Anuj J.

    2014-01-01

    Purpose: Understanding the radiation dose to a patient is essential when considering the use of an ionizing diagnostic imaging test for clinical diagnosis and screening. Using Monte Carlo simulations, the authors estimated the three-dimensional organ-dose distribution from neutron and gamma irradiation of the male liver, female liver, and female breasts for neutron- and gamma-stimulated spectroscopic imaging. Methods: Monte Carlo simulations were developed using the Geant4 GATE application and a voxelized XCAT human phantom. A male and a female whole body XCAT phantom was voxelized into 256 × 256 × 600 voxels (3.125 × 3.125 × 3.125 mm3). A monoenergetic rectangular beam of 5.0 MeV neutrons or 7.0 MeV photons was made incident on a 2 cm thick slice of the phantom. The beam was rotated at eight different angles around the phantom ranging from 0° to 180°. Absorbed dose was calculated for each individual organ in the body and dose volume histograms were computed to analyze the absolute and relative doses in each organ. Results: The neutron irradiations of the liver showed the highest organ dose absorption in the liver, with appreciably lower doses in other proximal organs. The dose distribution within the irradiated slice exhibited substantial attenuation with increasing depth along the beam path, attenuating to ∼15% of the maximum value at the beam exit side. The gamma irradiation of the liver imparted the highest organ dose to the stomach wall. The dose distribution from the gammas showed a region of dose buildup at the beam entrance, followed by a relatively uniform dose distribution to all of the deep tissue structures, attenuating to ∼75% of the maximum value at the beam exit side. For the breast scans, both the neutron and gamma irradiation registered maximum organ doses in the breasts, with all other organs receiving less than 1% of the breast dose. Effective doses ranged from 0.22 to 0.37 mSv for the neutron scans and 41 to 66 mSv for the gamma scans

  1. Low level measurement of (60)Co by gamma ray spectrometry using γ-γ coincidence.

    PubMed

    Paradis, H; de Vismes Ott, A; Luo, M; Cagnat, X; Piquemal, F; Gurriaran, R

    2016-03-01

    This paper presents the latest development of the laboratory to measure the natural and artificial massic activities in environmental samples. The measurement method of coincident emitters by gamma-gamma coincidence using an anti-Compton device and its digital electronics is described. Results obtained with environmental samples are shown. Despite its low efficiency, this method decreases detection limits of (60)Co for certain samples compared to conventional gamma-ray spectrometry due to its very low background. PMID:26682892

  2. High-Spin Gamma-Ray Spectroscopy in BISMUTH-198, Superdeformation in GOLD-191, and Multi-Photon Resonances in Low Energy Positron-Electron Scattering

    NASA Astrophysics Data System (ADS)

    Vo, Duc Ta.

    1993-01-01

    The properties of low-and high-spin levels in ^{198}Bi have been studied with the ^{181}Ta(^ {22}Ne,5n)^{198}Bi reaction at 116 MeV and 120 MeV bombarding energies. Levels along and near the yrast lines, including one isomer, were established up to spin J ~ 30hbar. The main configurations of these states are suggested to be pi h_{9/2} coupled to the known excited states in ^{197 }Pb. A sequence of states built on the excitation of the odd proton (coupled to one, two, or three quasi neutron-holes) was observed. In addition, at least two collective bands were observed. These two bands are backbending bands and are suggested to be oblate collective structures built on oblate proton and possibly neutron states. A superdeformed (SD) band was observed for the first time in an Au isotope. The reaction used was ^{11}B + ^{186 }W, demonstrating that very light ions can be used to populate SD bands at high angular momentum. The band is assigned to ^{191}Au. The gamma-ray energies are at the so -called quarter-point energies of the ^{192 }Hg SD band, indicating that the ^ {191}Au SD band is "identical" to that of ^{192}Hg. A search for resonant states in low-energy e ^+e^- scattering through their decay to multi-photon final states was performed using e ^+ from ^{68}Ga sources and a Pb absorber. Energy-sum and invariant mass spectra of coincident 2gamma and 3gamma events were obtained using the 20-element High Energy-Resolution Array (HERA) facility. No evidence for resonant states was found, and upper limits for the partial decay widths of such resonances were established in the energy range from 1.1 to 1.8 MeV.

  3. A label-free fluorescence strategy for selective detection of nicotinamide adenine dinucleotide based on a dumbbell-like probe with low background noise.

    PubMed

    Chen, Xuexu; Lin, Chunshui; Chen, Yiying; Wang, Yiru; Chen, Xi

    2016-03-15

    In this work we developed a novel label-free fluorescence sensing approach for the detection of nicotinamide adenine dinucleotide (NAD(+)) based on a dumbbell-like DNA probe designed for both ligation reaction and digestion reaction with low background noise. SYBR Green I (SG I), a double-helix dye, was chosen as the readout fluorescence signal. In the absence of NAD(+), the ligation reaction did not occur, but the probe was digested to mononucleotides after the addition of exonuclease I (Exo I) and exonuclease I (Exo III), resulting in a weak fluorescence intensity due to the weak interaction between SG I and mononucleotides. In the presence of NAD(+), the DNA probe was ligated by Escherichia coli DNA ligase, blocking the digestion by Exo I and Exo III. As a result, SG I was intercalated into the stem part of the DNA dumbbell probe and fluorescence enhancement was achieved. This method was simple in design, fast to operate, with good sensitivity and selectivity which could discriminate NAD(+) from its analogs. PMID:26454831

  4. A new method based on low background instrumental neutron activation analysis for major, trace and ultra-trace element determination in atmospheric mineral dust from polar ice cores.

    PubMed

    Baccolo, Giovanni; Clemenza, Massimiliano; Delmonte, Barbara; Maffezzoli, Niccolò; Nastasi, Massimiliano; Previtali, Ezio; Prata, Michele; Salvini, Andrea; Maggi, Valter

    2016-05-30

    Dust found in polar ice core samples present extremely low concentrations, in addition the availability of such samples is usually strictly limited. For these reasons the chemical and physical analysis of polar ice cores is an analytical challenge. In this work a new method based on low background instrumental neutron activation analysis (LB-INAA) for the multi-elemental characterization of the insoluble fraction of dust from polar ice cores is presented. Thanks to an accurate selection of the most proper materials and procedures it was possible to reach unprecedented analytical performances, suitable for ice core analyses. The method was applied to Antarctic ice core samples. Five samples of atmospheric dust (μg size) from ice sections of the Antarctic Talos Dome ice core were prepared and analyzed. A set of 37 elements was quantified, spanning from all the major elements (Na, Mg, Al, Si, K, Ca, Ti, Mn and Fe) to trace ones, including 10 (La, Ce, Nd, Sm, Eu, Tb, Ho, Tm, Yb and Lu) of the 14 natural occurring lanthanides. The detection limits are in the range of 10(-13)-10(-6) g, improving previous results of 1-3 orders of magnitude depending on the element; uncertainties lies between 4% and 60%. PMID:27154827

  5. A Micromegas-based low-background x-ray detector coupled to a slumped-glass telescope for axion research

    NASA Astrophysics Data System (ADS)

    Aznar, F.; Castel, J.; Christensen, F. E.; Dafni, T.; Decker, T. A.; Ferrer-Ribas, E.; Garcia, J. A.; Giomataris, I.; Garza, J. G.; Hailey, C. J.; Hill, R. M.; Iguaz, F. J.; Irastorza, I. G.; Jakobsen, A. C.; Luzon, G.; Mirallas, H.; Papaevangelou, T.; Pivovaroff, M. J.; Ruz, J.; Vafeiadis, T.; Vogel, J. K.

    2015-12-01

    We report on the design, construction and operation of a low background x-ray detection line composed of a shielded Micromegas detector of the microbulk technology. The detector is made from radiopure materials and is placed at the focal point of a ~ 5 cm diameter, 1.5 m focal-length, cone-approximation Wolter I x-ray telescope (XRT) assembled from thermally-formed (or "slumped") glass substrates deposited with multilayer coatings. The system has been conceived as a technological pathfinder for the future International Axion Observatory (IAXO), as it combines two of the techniques (optic and detector) proposed in the conceptual design of the project. It is innovative for two reasons: it is the first time an x-ray optic has been designed and fabricated specifically for axion research, and the first time a Micromegas detector has been operated with an x-ray optic. The line has been installed at one end of the CERN Axion Solar Telescope (CAST) magnet and is currently looking for solar axions. The combination of the XRT and Micromegas detector provides the best signal-to-noise ratio obtained so far by any detection system of the CAST experiment with a background rate of 5.4×10-3 counts per hour in the energy region-of-interest and signal spot area.

  6. Exploring the Impact of Nuclear Data Uncertainties in Ultra-high Resolution Gamma Spectroscopy for Isotopic Analysis Using Approximate Bayesian Computation

    SciTech Connect

    Burr, T.; Hoover, A.; Croft, S.; Rabin, M.

    2015-01-15

    High purity germanium (HPGe) currently provides the highest readily available resolution gamma detection for a broad range of radiation measurements, but microcalorimetry is a developing option that has considerably higher resolution even than HPGe. Superior microcalorimetry resolution offers the potential to better distinguish closely spaced X-rays and gamma-rays, a common challenge for the low energy spectral region near 100 keV from special nuclear materials, and the higher signal-to-background ratio also confers an advantage in detection limit. As microcalorimetry continues to develop, it is timely to assess the impact of uncertainties in detector and item response functions and in basic nuclear data, such as branching ratios and half-lives, used to interpret spectra in terms of the contributory radioactive isotopes. We illustrate that a new inference option known as approximate Bayesian computation (ABC) is effective and convenient both for isotopic inference and for uncertainty quantification for microcalorimetry. The ABC approach opens a pathway to new and more powerful implementations for practical applications than currently available.

  7. Analysis of gamma-irradiated melon, pumpkin, and sunflower seeds by electron paramagnetic resonance spectroscopy and gas chromatography-mass spectrometry.

    PubMed

    Sin, Della W M; Wong, Yiu Chung; Yao, Wai Yin

    2006-09-20

    Seeds of melon (Citrullus lanatus var. sp.), pumpkin (Cucurbita moschata), and sunflower (Heliantus annus) were gamma-irradiated at 1, 3, 5, and 10 kGy and analyzed by electron paramagnetic resonance (EPR) and gas chromatography-mass spectrometry (GC-MS) according to EN1787:2000 and EN1785:2003, respectively. Distinguishable triplet signals due to the presence of induced cellulose radicals were found at 2.0010-2.0047 g in the EPR spectra. The gamma-irradiated radiolytic markers of 2-dodecylcyclobutanone (2-DCB) and 2-tetradecylcyclobutanone (2-TCB) were identified in all irradiated seed samples. Both the free radicals and the alkylcyclobutanones were found to increase with irradiation dose. In general, linear relationships between the amount of radicals and irradiation dosage could be established. Studies at an ambient temperature (20-25 degrees C) in a humidity-controlled environment showed a complete disappearance of the cellulosic peaks for irradiated samples upon 60 days of storage. Such instability behavior was considered to render the usefulness of using EPR alone in the determination of irradiated seed samples. On the other hand, 2-DCB and 2-TCB were also found to decompose rapidly (>85% loss after 120 days of storage), but the radiolytic markers remained quantifiable after 120 days of postirradiation storage. These results suggest that GC-MS is a versatile and complimentary technique for the confirmation of irradiation treatment to seeds. PMID:16968077

  8. High-precision gamma-ray spectroscopy of 82Rb and 72As, two important medical isotopes used in positron emission tomography

    NASA Astrophysics Data System (ADS)

    Nino, Michael; McCutchan, E.; Smith, S.; Sonzogni, A.; Muench, L.; Greene, J.; Carpenter, M.; Zhu, S.; Lister, C.

    2015-10-01

    Both 82Rb and 72As are very important medical isotopes used in imaging procedures, yet their full decay schemes were last studied decades ago using low-sensitivity detection systems; high quality decay data is necessary to determine the total dose received by the patient, the background in imaging technologies, and shielding requirements in production facilities. To improve the decay data of these two isotopes, sources were produced at the Brookhaven Linac Isotope Producer (BLIP) and then the Gammasphere array, consisting of 89 Compton-suppressed HPGe detectors, at Argonne National Laboratory was used to analyze the gamma-ray emissions from the daughter nuclei 82 Kr and 72 Ge. Gamma-ray singles and coincidence information were recorded and analyzed using Radware Gf3m software. Significant revisions were made to the level schemes including the observation of many new transitions and levels as well as a reduction in uncertainty on measured γ-ray intensities and deduced β-feedings. The new decay schemes as well as their impact on dose calculations will be presented. DOE Isotope Program is acknowledged for funding ST5001030. Work supported by the U.S. DOE under Grant No. DE-FG02-94ER40848 and Contract Nos. DE-AC02-98CH10946 and DE-AC02-06CH11357 and by the Science Undergraduate Laboratory Internships Program (SULI).

  9. Basic characterization of highly enriched uranium by gamma spectrometry

    NASA Astrophysics Data System (ADS)

    Nguyen, Cong Tam; Zsigrai, József

    2006-05-01

    Gamma-spectrometric methods suitable for the characterization of highly enriched uranium samples encountered in illicit trafficking of nuclear materials are presented. In particular, procedures for determining the 234U, 235U, 238U, 232U and 236U contents and the age of highly enriched uranium are described. Consequently, the total uranium content and isotopic composition can be calculated. For determining the 238U and 232U contents a low-background chamber was used. In addition, age dating of uranium was also performed using low-background spectrometry.

  10. X-ray remote sensing and in-situ spectroscopy for planetary exploration missions and gamma-ray remote sensing and in-situ spectroscopy for planetary exploration missions

    NASA Technical Reports Server (NTRS)

    Mahdavi, M.; Giboni, K. L.; Vajda, S.; Schweitzer, J.

    1994-01-01

    Detectors that will be used for planetary missions must have their responses calibrated in a reproducible manner. A calibration facility is being constructed at Schlumberger-Doll Research for gamma and x ray detectors. With this facility the detector response can be determined in an invariant and reproducible fashion. Initial use of the facility is expected for the MARS94 detectors. Work is continuing to better understand the rare earth oxyorthosilicates and to define their characteristics. This will allow a better use of these scintillators for planetary missions. In a survey of scintillating materials two scintillators were identified as promising candidates besides GSO, LSO, and YSO. These are CdWO4 and CsI(Tl). It will be investigated if a detector with a better overall performance can be assembled with various photon converters. Considerable progress was achieved in photomultiplier design. The length of an 1 inch diameter PMT could be reduced from 4.2 to 2.5 inches without performance degradation. This technology is being employed in the gamma ray detector for the NEAR project. A further weight and size reduction of the detector package can be achieved with miniaturized integrated power supplies.

  11. DNA repair by photolyase: a novel substrate with low background absorption around 265 nm for transient absorption studies in the UV.

    PubMed

    Thiagarajan, Viruthachalam; Villette, Sandrine; Espagne, Agathe; Eker, Andre P M; Brettel, Klaus; Byrdin, Martin

    2010-01-19

    CPD photolyase enzymatically repairs the major UV-induced lesion in DNA, the cyclobutane pyrimidine dimer (CPD), by photoreversion of the damage reaction. An enzyme-bound reduced flavin (FADH(-)) cofactor functions as photosensitizer. Upon excitation, it transiently transfers an electron to the CPD, triggering scission of the interpyrimidine bonds. After repair completion, the electron returns to the flavin to restore its functional reduced form. A major difficulty for time-resolved spectroscopic monitoring of the enzymatic repair reaction is that absorption changes around 265 nm accompanying pyrimidine restoration are obscured by the strong background absorption of the nondimerized bases in DNA. Here we present a novel substrate for CPD photolyase that absorbs only weakly around 265 nm: a modified thymidine 10-mer with a central CPD and all bases, except the one at the 3' end, replaced by 5,6-dihydrothymine which virtually does not absorb around 265 nm. Repair of this substrate by photolyases from Anacystis nidulans and from Escherichia coli was compared with repair of two conventional substrates: a 10-mer of unmodified thymidines containing a central CPD and an acetone-sensitized thymidine 18-mer that contained in average six randomly distributed CPDs per strand. In all cases, the novel substrate was repaired with an efficiency very similar to that of the conventional substrates (quantum yields in the order of 0.5 upon excitation of FADH(-)). Flash-induced transient absorption changes at 267 nm could be recorded on a millisecond time scale with a single subsaturating flash and yielded very similar signals for all three substrates. Because of its low background absorption around 265 nm and the defined structure, the novel substrate is a promising tool for fast and ultrafast transient absorption studies on pyrimidine dimer splitting by CPD photolyase. PMID:20000331

  12. Optimal bandgap variants of Cd 1- xZn xTe for high-resolution X-ray and gamma-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Toney, J. E.; Schlesinger, T. E.; James, R. B.

    1999-06-01

    We show that the trade-off between noise and charge generation statistics in Cd 1- xZn xTe leads to an optimal band gap of approximately 2.0 eV at room temperature. This implies a ZnTe fraction of approximately 0.7-0.8. We show that for X-rays and relatively low energy gamma-rays Cd 0.2Zn 0.8Te theoretically offers a significant potential improvement in energy resolution over Cd 0.9Zn 0.1Te even if compensation of shallow levels is less complete and carrier lifetimes are an order of magnitude lower for the higher x variant. We also show that these calculations are consistent with observed detector performance reported by many workers over a large period of time.

  13. Gamma Ray Astronomy

    NASA Technical Reports Server (NTRS)

    Wu, S. T.

    2000-01-01

    The project has progressed successfully during this period of performance. The highlights of the Gamma Ray Astronomy teams efforts are: (1) Support daily BATSE data operations, including receipt, archival and dissemination of data, quick-look science analysis, rapid gamma-ray burst and transient monitoring and response efforts, instrument state-of-health monitoring, and instrument commanding and configuration; (2) On-going scientific analysis, including production and maintenance of gamma-ray burst, pulsed source and occultation source catalogs, gamma-ray burst spectroscopy, studies of the properties of pulsars and black holes, and long-term monitoring of hard x-ray sources; (3) Maintenance and continuous improvement of BATSE instrument response and calibration data bases; (4) Investigation of the use of solid state detectors for eventual application and instrument to perform all sky monitoring of X-Ray and Gamma sources with high sensitivity; and (5) Support of BATSE outreach activities, including seminars, colloquia and World Wide Web pages. The highlights of this efforts can be summarized in the publications and presentation list.

  14. Investigation of (235)U, (226)Ra, (232)Th, (40)K, (137)Cs, and heavy metal concentrations in Anzali international wetland using high-resolution gamma-ray spectrometry and atomic absorption spectroscopy.

    PubMed

    Zare, Mohammad Reza; Kamali, Mahdi; Fallahi Kapourchali, Maryam; Bagheri, Hashem; Khoram Bagheri, Mahdi; Abedini, Ali; Pakzad, Hamid Reza

    2016-02-01

    Measurements of natural radioactivity levels and heavy metals in sediment and soil samples of the Anzali international wetland were carried out by two HPGe-gamma ray spectrometry and atomic absorption spectroscopy techniques. The concentrations of (235)U, (226)Ra, (232)Th, (40)K, and (137)Cs in sediment samples ranged between 1.05 ± 0.51-5.81 ± 0.61, 18.06 ± 0.63-33.36 ± .0.34, 17.57 ± 0.38-45.84 ± 6.23, 371.88 ± 6.36-652.28 ± 11.60, and 0.43 ± 0.06-63.35 ± 0.94 Bq/kg, while in the soil samples they vary between 2.36-5.97, 22.71-38.37, 29.27-42.89, 472.66-533, and 1.05-9.60 Bq/kg for (235)U, (226)Ra, (232)Th, (40)K, and (137)Cs, respectively. Present results are compared with the available literature data and also with the world average values. The radium equivalent activity was well below the defined limit of 370 Bq/kg. The external hazard indices were found to be less than 1, indicating a low dose. Heavy metal concentrations were found to decrease in order as Fe > Mn > Sr > Zn > Cu > Cr > Ni > Pb > Co > Cd. These measurements will serve as background reference levels for the Anzali wetland. PMID:26490904

  15. Photometry and spectroscopy of GRB 060526: a detailed study of the afterglow and host galaxy of a z = 3.2 gamma-ray burst

    NASA Astrophysics Data System (ADS)

    Thöne, C. C.; Kann, D. A.; Jóhannesson, G.; Selj, J. H.; Jaunsen, A. O.; Fynbo, J. P. U.; Akerlof, C. W.; Baliyan, K. S.; Bartolini, C.; Bikmaev, I. F.; Bloom, J. S.; Burenin, R. A.; Cobb, B. E.; Covino, S.; Curran, P. A.; Dahle, H.; Ferrero, A.; Foley, S.; French, J.; Fruchter, A. S.; Ganesh, S.; Graham, J. F.; Greco, G.; Guarnieri, A.; Hanlon, L.; Hjorth, J.; Ibrahimov, M.; Israel, G. L.; Jakobsson, P.; Jelínek, M.; Jensen, B. L.; Jørgensen, U. G.; Khamitov, I. M.; Koch, T. S.; Levan, A. J.; Malesani, D.; Masetti, N.; Meehan, S.; Melady, G.; Nanni, D.; Näränen, J.; Pakstiene, E.; Pavlinsky, M. N.; Perley, D. A.; Piccioni, A.; Pizzichini, G.; Pozanenko, A.; Roming, P. W. A.; Rujopakarn, W.; Rumyantsev, V.; Rykoff, E. S.; Sharapov, D.; Starr, D.; Sunyaev, R. A.; Swan, H.; Tanvir, N. R.; Terra, F.; de Ugarte Postigo, A.; Vreeswijk, P. M.; Wilson, A. C.; Yost, S. A.; Yuan, F.

    2010-11-01

    Aims: With this paper we want to investigate the highly variable afterglow light curve and environment of gamma-ray burst (GRB) 060526 at z = 3.221. Methods: We present one of the largest photometric datasets ever obtained for a GRB afterglow, consisting of multi-color photometric data from the ultraviolet to the near infrared. The data set contains 412 data points in total to which we add additional data from the literature. Furthermore, we present low-resolution high signal-to-noise spectra of the afterglow. The afterglow light curve is modeled with both an analytical model using broken power law fits and with a broad-band numerical model which includes energy injections. The absorption lines detected in the spectra are used to derive column densities using a multi-ion single-component curve-of-growth analysis from which we derive the metallicity of the host of GRB 060526. Results: The temporal behaviour of the afterglow follows a double broken power law with breaks at t = 0.090 ± 0.005 and t = 2.401 ± 0.061 days. It shows deviations from the smooth set of power laws that can be modeled by additional energy injections from the central engine, although some significant microvariability remains. The broadband spectral-energy distribution of the afterglow shows no significant extinction along the line of sight. The metallicity derived from S ii and Fe ii of [S/H] = -0.57 ± 0.25 and [Fe/H] = -1.09 ± 0.24 is relatively high for a galaxy at that redshift but comparable to the metallicity of other GRB hosts at similar redshifts. At the position of the afterglow, no host is detected to F775W(AB) = 28.5 mag with the HST, implying an absolute magnitude of the host M(1500 Å) > -18.3 mag which is fainter than most long-duration hosts, although the GRB may be associated with a faint galaxy at a distance of 11 kpc. Based in part on observations obtained with the European Southern Observatory's Very Large Telescope under proposals 077.D-0661 (PI: Vreeswijk) and 177.A-0591

  16. Polonium-Lead Extractions to Determine the Best Method for the Quantification of Clean Lead Used in Low-Background Radiation Detectors

    SciTech Connect

    Miley, Sarah M.; Payne, Rosara F.; Schulte, Shannon M.; Finn, Erin C.

    2009-12-01

    Radiation detectors used to search for the existence of exceptionally rare phenomena, such as double-beta decay and dark matter interactions, as well as tiny traces of environmental radioactivity, require the elimination of background signals. Modern detection systems created from ultra pure materials and operated deep underground may be sensitive enough to "see" these rare phenomena, but background activity in Pb gamma-ray shielding could still be a critical stumbling block owing to alpha and beta emissions of Pb, Bi, and Po in the mass 210 chain. To minimize the probability of overwhelming activity from Pb, the alpha activity of 210Pb is quantified. However, a reliable quantification procedure that does not require large volumes of chemicals has not yet been established. Two procedures created for this purpose have been tested for the quantification of alpha activity in lead. Both procedures were designed to start with less than 10g Pb samples to reduce reagents needed and combined precipitation with column separation to isolate 210Pb, followed by alpha spectrometry. One procedure shows promise for obtaining high recoveries and good separation.

  17. Gamma-spectrometric uranium age-dating using intrinsic efficiency calibration

    NASA Astrophysics Data System (ADS)

    Nguyen, Cong Tam; Zsigrai, József

    2006-01-01

    A non-destructive, gamma-spectrometric method for uranium age-dating is presented which is applicable to material of any physical form and geometrical shape. It relies on measuring the daughter/parent activity ratio 214Bi/234U by low-background, high-resolution gamma-spectrometry using intrinsic efficiency calibration. The method does not require the use of any reference materials nor the use of an efficiency calibrated geometry.

  18. Gamma Knife

    MedlinePlus

    ... results are sent to the Gamma Knife®'s planning computer system. Together, physicians ( radiation oncologists and neurosurgeons) and medical physicists delineate targets and normal anatomical structures. They use a planning computer program to determine the exact spatial relationship between ...

  19. Gamma watermarking

    DOEpatents

    Ishikawa, Muriel Y.; Wood, Lowell L.; Lougheed, Ronald W.; Moody, Kenton J.; Wang, Tzu-Fang

    2004-05-25

    A covert, gamma-ray "signature" is used as a "watermark" for property identification. This new watermarking technology is based on a unique steganographic or "hidden writing" digital signature, implemented in tiny quantities of gamma-ray-emitting radioisotopic material combinations, generally covertly emplaced on or within an object. This digital signature may be readily recovered at distant future times, by placing a sensitive, high energy-resolution gamma-ray detecting instrument reasonably precisely over the location of the watermark, which location may be known only to the object's owner; however, the signature is concealed from all ordinary detection means because its exceedingly low level of activity is obscured by the natural radiation background (including the gamma radiation naturally emanating from the object itself, from cosmic radiation and material surroundings, from human bodies, etc.). The "watermark" is used in object-tagging for establishing object identity, history or ownership. It thus may serve as an aid to law enforcement officials in identifying stolen property and prosecuting theft thereof. Highly effective, potentially very low cost identification-on demand of items of most all types is thus made possible.

  20. Low-background trace-gas detector

    NASA Technical Reports Server (NTRS)

    Rosengren, L.

    1978-01-01

    Spectrophone detects very small concentrations of trace gases. With gas in sample cell, laser is tuned to absorption line of interest. Molecular absorption in cell produces pulsed acoustical pressure at chopper frequency. Two optical paths with very different absorption lengths are used to pretune cell to balance out background absorption by cell windows.

  1. Gamma Ray Imaging for Environmental Remediation

    SciTech Connect

    Johnson, W. Neil; Luke, Paul N.; Kurfess, J.D.; Phlips, Bernard F.; Kroeger, R.A.; Phillips, G.W.

    1999-06-01

    The goal of this project is the development of field portable gamma-ray detectors that can both image gamma rays from radioactive emission and determine the isotopic composition by the emitted spectrum. Most instruments to date have had either very good imaging with no spectroscopy, or very good spectroscopy with no imaging. The only instruments with both imaging and spectroscopy have had rather poor quality imaging and spectroscopy (e.g. NaI Anger Cameras). The technology would have widespread applications, from laboratory nuclear physics, to breast cancer imaging, to astronomical research. For this project, we focus on the applications in the field of fissile materials, spent nuclear fuels and decontamination and decommissioning.

  2. Gamma-Ray Pulse Tube Cooler Development and Testing

    NASA Technical Reports Server (NTRS)

    Ross, R.; Johnson, D.; Kotsubo, V.; Evtimov, B.; Olson, J.; Nast, T.; Rawlings, R.

    2000-01-01

    For a variety of space-science applications, such as gamma-ray spectroscopy, the introduction of cryogenic cooling via a cryocooler can greatly increase the potential science return by allowing the use of more sensitive and lower noise detectors.

  3. Extended use of alanine irradiated in experimental reactor for combined gamma- and neutron-dose assessment by ESR spectroscopy and thermal neutron fluence assessment by measurement of (14)C by LSC.

    PubMed

    Bartoníček, B; Kučera, J; Světlík, I; Viererbl, L; Lahodová, Z; Tomášková, L; Cabalka, M

    2014-11-01

    Gamma- and neutron doses in an experimental reactor were measured using alanine/electron spin resonance (ESR) spectrometry. The absorbed dose in alanine was decomposed into contributions caused by gamma and neutron radiation using neutron kerma factors. To overcome a low sensitivity of the alanine/ESR response to thermal neutrons, a novel method has been proposed for the assessment of a thermal neutron flux using the (14)N(n,p) (14)C reaction on nitrogen present in alanine and subsequent measurement of (14)C by liquid scintillation counting (LSC). PMID:24581599

  4. Quarkonium spectroscopy

    SciTech Connect

    Scharre, D.L.

    1981-06-01

    Recent experimental investigations of heavy quark-antiquark bound state systems are reviewed. Results from SPEAR on charmonium spectroscopy and from DORIS and CESR on bottomonium spectroscopy are presented. The current status of the search for top is also discussed.

  5. Gamma Ray Imaging for Environmental Remediation

    SciTech Connect

    B.F. Philips; R.A. Kroeger: J.D. Kurfess: W.N. Johnson; E.A. Wulf; E. I. Novikova

    2004-11-12

    This program is the development of germanium strip detectors for environmental remediation. It is a collaboration between the Naval Research Laboratory and Lawrence Berkeley National Lab. The goal is to develop detectors that are simultaneously capable of excellent spectroscopy and imaging of gamma radiation.

  6. The gamma irradiation effects on structural and optical properties of silk fibroin/HPMC blend films

    NASA Astrophysics Data System (ADS)

    Shetty, G. Rajesha; Rao, B. Lakshmeesha; Gowda, Mahadeva; Shivananda, C. S.; Asha, S.; Byrappa, K.; Sangappa, Y.

    2016-05-01

    In this paper the structural, chemical and optical properties of gamma irradiated silk fibroin/Hydroxypropyl methyl cellulose (SF-HPMC) blend films were studied using X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR) and UV-visible spectroscopy. The results indicate that the gamma radiation did not affect significantly the primary structure of polypeptide arrangement in the blend films. But the optical properties of the blends changed with gamma irradiation dosage.

  7. Neutron capture by Ru: Neutron cross sections of {sup 96,102,104}Ru and gamma-ray spectroscopy in the decays of {sup 97,103,105}Ru

    SciTech Connect

    Krane, K. S.

    2010-04-15

    Cross sections for radiative capture of neutrons have been measured for stable isotopes of Ru with mass numbers 96,102, and 104. From separate irradiations using thermal and epithermal neutrons, independent values for the thermal cross section and effective resonance integral have been determined. Spectroscopic studies of the gamma rays emitted in the decays of {sup 97,103,105}Ru have enabled improvements in the precision of the energies and intensities of the radiations along with corresponding improvements in the beta-decay feeding intensities and the energies of the levels in the respective daughter nuclei. Similar spectroscopic measurements of the decays of {sup 105}Rh (daughter of {sup 105}Ru) and {sup 96}Tc (produced from n,p reactions on {sup 96}Ru) have resulted in improved gamma-ray energies and intensities in those decays.

  8. Gamma-ray constraints on supernova nucleosynthesis

    NASA Technical Reports Server (NTRS)

    Leising, Mark D.

    1994-01-01

    Gamma-ray spectroscopy holds great promise for probing nucleosynthesis in individual supernova explosions via short-lived radioactivity, and for measuring current global Galactic supernova nucleosynthesis with longer-lived radioactivity. It was somewhat surprising that the former case was realized first for a Type II supernova, when both Co-56 and Co-57 were detected in SN 1987A. These provide unprecedented constraints on models of Type II explosions and nucleosynthesis. Live Al-26 in the Galaxy might come from Type II supernovae, and if it is eventually shown to be so, can constrain massive star evolution, supernova nucleosynthesis, and the Galactic Type II supernova rate. Type Ia supernovae, thought to be thermonuclear explosions, have not yet been detected in gamma-rays. This is somewhat surprising given current models and recent Co-56 detection attempts. Ultimately, gamma-ray measurements can confirm their thermonuclear nature, probe the nuclear burning conditions, and help evaluate their contributions to Galactic nucleosynthesis. Type Ib/c supernovae are poorly understood. Whether they are core collapse or thermonuclear events might be ultimately settled by gamma-ray observations. Depending on details of the nuclear processing, any of these supernova types might contribute to a detectable diffuse glow of Fe-60 gamma-ray lines. Previous attempts at detection have come very close to expected emission levels. Remnants of any type of age less that a few centuries might be detectable as individual spots of Ti-44 gamma-ray line emission. It is in fact quite surprising that previous surveys have not discovered such spots, and the constraints on the combination of nucleosynthesis yields and supernova rates are very interesting. All of these interesting limits and possibilities mean that the next mission, International Gamma-Ray Astrophysics Laboratory (INTEGRAL), if it has sufficient sensitivity, is very likely to lead to the realization of much of the great potential

  9. Mossbauer Spectroscopy.

    ERIC Educational Resources Information Center

    Stevens, John G.; Bowen, Lawrence H.

    1980-01-01

    Reviews current research in Mossbauer spectroscopy, including instrumentation and experimental techniques, spectral analysis, catalysts and surfaces, environmental studies, medical applications and atmospheric air studies. Cites 346 references. (CS)

  10. Gamma ray generator

    DOEpatents

    Firestone, Richard B; Reijonen, Jani

    2014-05-27

    An embodiment of a gamma ray generator includes a neutron generator and a moderator. The moderator is coupled to the neutron generator. The moderator includes a neutron capture material. In operation, the neutron generator produces neutrons and the neutron capture material captures at least some of the neutrons to produces gamma rays. An application of the gamma ray generator is as a source of gamma rays for calibration of gamma ray detectors.

  11. Raman Spectroscopy.

    ERIC Educational Resources Information Center

    Gerrard, Donald L.

    1984-01-01

    Reviews literature on Raman spectroscopy from late 1981 to late 1983. Topic areas include: instrumentation and sampling; liquids and solutions; gases and matrix isolation; biological molecules; polymers; high-temperature and high-pressure studies; Raman microscopy; thin films and surfaces; resonance-enhanced and surface-enhanced spectroscopy; and…

  12. Sub-nanosecond Half-life Measurement of the Yrast I{sup π}=5{sup −} State in the N=78 Nucleus {sup 136}{sub 58}Ce using Fast-timing Coincident Gamma-ray Spectroscopy

    SciTech Connect

    Alharbi, T.; Regan, P.H.; Mărginean, N.; Podolyák, Zs.; Bajoga, A.; Britton, R.; Bucurescu, D.; Deleanu, D.; Filipescu, D.; Ghită, D.; Glodariu, T.; Mihai, C.; Mulholland, K.; Mărginean, R.; Negret, A.; Nita, C.R.; Patel, Z.; Roberts, O.J.; Stroe, L.; Sava, T.; and others

    2014-06-15

    We report on the measurement of the half-life of the yrast I{sup π}=5{sup −} state in the transitional nucleus {sup 136}Ce using a combined HPGe-LaBr3(Ce) scintillator gamma-ray detection array. The measured value for the E1 decay is approximately half a nanosecond, which corresponds to an E1 decay strength of approximately 2×10{sup −6} Wu. This value is in line with single-particle type E1 decays in this mass region and suggests no sign of additional K-hindrance associated with axially symmetric quadrupole deformations observed for lighter cerium isotopes.

  13. The gamma-ray telescope Gamma-1

    NASA Technical Reports Server (NTRS)

    Akimov, V. V.; Nesterov, V. E.; Rodin, V. G.; Kalinkin, L. F.; Balibanov, V. M.; Prilutsky, O. F.; Leikov, N. G.; Bielaoussov, A. S.; Dobrian, L. B.; Poluektov, V. P.

    1985-01-01

    French and Soviet specialists have designed and built the gamma-ray telescope GAMMA-1 to detect cosmic gamma rays above 50 MeV. The sensitive area of the detector is 1400 sq cm, energy resolution is 30% at 300 MeV, and angular resolution 1.2 deg at 300 MeV (and less than 20' arc when a coded aperture mask is used). Results on calibration of the qualification model and Monte-Carlo calculations are presented.

  14. Gamma ray astrophysics to the year 2000. Report of the NASA Gamma Ray Program Working Group

    NASA Technical Reports Server (NTRS)

    1988-01-01

    Important developments in gamma-ray astrophysics up to energies of 100 GeV during the last decade are reviewed. Also, the report seeks to define the major current scientific goals of the field and proposes a vigorous program to pursue them, extending to the year 2000. The goals of gamma-ray astronomy include the study of gamma rays which provide the most direct means of studying many important problems in high energy astrophysics including explosive nucleosynthesis, accelerated particle interactions and sources, and high-energy processes around compact objects. The current research program in gamma-ray astronomy in the U.S. including the space program, balloon program and foreign programs in gamma-ray astronomy is described. The high priority recommendations for future study include an Explorer-class high resolution gamma-ray spectroscopy mission and a Get Away Special cannister (GAS-can) or Scout class multiwavelength experiment for the study of gamma-ray bursts. Continuing programs include an extended Gamma Ray Observatory mission, continuation of the vigorous program of balloon observations of the nearby Supernova 1987A, augmentation of the balloon program to provide for new instruments and rapid scientific results, and continuation of support for theoretical research. Long term recommendations include new space missions using advanced detectors to better study gamma-ray sources, the development of these detectors, continued study for the assembly of large detectors in space, collaboration with the gamma-ray astronomy missions initiated by other countries, and consideration of the Space Station attached payloads for gamma-ray experiments.

  15. A Correlated Optical and Gamma Emission from GRB 081126A

    SciTech Connect

    Gendre, B.; Klotz, A.; Atteia, J. L.; Boeer, M.; Coward, D. M.; Imerito, A. C.

    2010-10-15

    We present an analysis of time-resolved optical emissions observed from the gamma-ray burst GRB 081126 during the prompt phase. The analysis employed time-resolved photometry using optical data obtained by the TAROT telescope, BAT data from the Swift spacecraft and time-resolved spectroscopy at high energies from the GBM instrument onboard the Fermi spacecraft. The optical emission of GRB 081126 is found to be compatible with the second gamma emission pulse shifted by a positive time-lag of 8.4{+-}3.9 sec. This is the first well resolved observation of a time lag between optical and gamma emissions during a gamma-ray burst. Our observations could potentially provide new constraints on the fireball model for gamma ray burst early emissions. Furthermore, observations of time-lags between optical and gamma ray photons provides an exciting opportunity to constrain quantum gravity theories.

  16. Fermi GBM Observations of Terrestrial Gamma Flashes

    NASA Technical Reports Server (NTRS)

    Wilson-Hodge, Colleen A.; Briggs, M. S.; Connaughton, V.; Fishman, G. J.; Bhat, P. N.; Paciesas, W. S.; Preece, R. D.; Kippen, R. M.; vonKienlin, A.; Dwyer, J. R.; Smith, D. M.; Holzworth, R.

    2010-01-01

    In its first two years of operation, the Fermi Gamma Ray Burst Monitor (GBM) has observed 79 Terrestrial Gamma Flashes (TGFs). The thick Bismuth Germanate (BGO) detectors are excellent for TGF spectroscopy, having a high probability of recording the full energy of an incident photon, spanning a broad energy range from 150 keV to 40 MeV, and recording a large number of photons per TGF. Correlations between GBM TGF triggers and lightning sferics detected with the World-Wide Lightning Location Network indicate that TGFs and lightning are simultaneous to within tens of microseconds.

  17. gamma-Hexachlorocyclohexane (gamma-HCH)

    Integrated Risk Information System (IRIS)

    gamma - Hexachlorocyclohexane ( gamma - HCH ) ; CASRN 58 - 89 - 9 Human health assessment information on a chemical substance is included in the IRIS database only after a comprehensive review of toxicity data , as outlined in the IRIS assessment development process . Sections I ( Health Hazard Asse

  18. Experimental set-up and optimization of a gamma-ray spectrometer for measurement of cosmogenic radionuclides in meteorites

    NASA Astrophysics Data System (ADS)

    Taricco, C.; Bhandari, N.; Colombetti, P.; Verma, N.; Vivaldo, G.

    2007-03-01

    We have developed a highly efficient and selective gamma-ray spectrometer with extremely low background for activity measurement of gamma emitting cosmogenic radionuclides in meteorites. This spectrometer can operate in specific modes to match decay scheme of a particular radionuclide and is specially suited for measurement of positron emitters. The system consists of a hyperpure Ge detector (3 kg, 147% relative efficiency), operating in coincidence with an umbrella of NaI(Tl) scintillator (90 kg) in order to achieve low background. The system is tuned such that strong interference due to naturally occurring uranium daughters, e.g. 214Bi present in the meteorites and in the laboratory environment, is minimized. It enables us to measure 44Ti (T=59.2y) which is ideal for studying centennial scale variations of cosmic ray flux in the interplanetary space with good reliability. The specific configuration of the coincidence system and electronics are described here.

  19. Gamma ray detector shield

    DOEpatents

    Ohlinger, R.D.; Humphrey, H.W.

    1985-08-26

    A gamma ray detector shield comprised of a rigid, lead, cylindrical-shaped vessel having upper and lower portions with an pneumatically driven, sliding top assembly. Disposed inside the lead shield is a gamma ray scintillation crystal detector. Access to the gamma detector is through the sliding top assembly.

  20. Gamma-Ray Library and Uncertainty Analysis: Passively Emitted Gamma Rays Used in Safeguards Technology

    SciTech Connect

    Parker, W

    2009-09-18

    Non-destructive gamma-ray analysis is a fundamental part of nuclear safeguards, including nuclear energy safeguards technology. Developing safeguards capabilities for nuclear energy will certainly benefit from the advanced use of gamma-ray spectroscopy as well as the ability to model various reactor scenarios. There is currently a wide variety of nuclear data that could be used in computer modeling and gamma-ray spectroscopy analysis. The data can be discrepant (with varying uncertainties), and it may difficult for a modeler or software developer to determine the best nuclear data set for a particular situation. To use gamma-ray spectroscopy to determine the relative isotopic composition of nuclear materials, the gamma-ray energies and the branching ratios or intensities of the gamma-rays emitted from the nuclides in the material must be well known. A variety of computer simulation codes will be used during the development of the nuclear energy safeguards, and, to compare the results of various codes, it will be essential to have all the {gamma}-ray libraries agree. Assessing our nuclear data needs allows us to create a prioritized list of desired measurements, and provides uncertainties for energies and especially for branching intensities. Of interest are actinides, fission products, and activation products, and most particularly mixtures of all of these radioactive isotopes, including mixtures of actinides and other products. Recent work includes the development of new detectors with increased energy resolution, and studies of gamma-rays and their lines used in simulation codes. Because new detectors are being developed, there is an increased need for well known nuclear data for radioactive isotopes of some elements. Safeguards technology should take advantage of all types of gamma-ray detectors, including new super cooled detectors, germanium detectors and cadmium zinc telluride detectors. Mixed isotopes, particularly mixed actinides found in nuclear reactor

  1. Covariance Analysis of Gamma Ray Spectra

    SciTech Connect

    Trainham, R.; Tinsley, J.

    2013-01-01

    The covariance method exploits fluctuations in signals to recover information encoded in correlations which are usually lost when signal averaging occurs. In nuclear spectroscopy it can be regarded as a generalization of the coincidence technique. The method can be used to extract signal from uncorrelated noise, to separate overlapping spectral peaks, to identify escape peaks, to reconstruct spectra from Compton continua, and to generate secondary spectral fingerprints. We discuss a few statistical considerations of the covariance method and present experimental examples of its use in gamma spectroscopy.

  2. Covariance analysis of gamma ray spectra

    SciTech Connect

    Trainham, R.; Tinsley, J.

    2013-01-15

    The covariance method exploits fluctuations in signals to recover information encoded in correlations which are usually lost when signal averaging occurs. In nuclear spectroscopy it can be regarded as a generalization of the coincidence technique. The method can be used to extract signal from uncorrelated noise, to separate overlapping spectral peaks, to identify escape peaks, to reconstruct spectra from Compton continua, and to generate secondary spectral fingerprints. We discuss a few statistical considerations of the covariance method and present experimental examples of its use in gamma spectroscopy.

  3. Measurement of cross sections for the 63Cu(alpha,gamma)67Ga reaction from 5.9-8.7 MeV

    SciTech Connect

    Basunia, M. Shamsuzzoha; Norman, Eric B.; Shugart, Howard A.; Smith, Alan R.; Dolinski, Michelle J.; Quiter, Brian J.

    2004-09-23

    We have measured cross sections for the 63Cu(alpha,gamma)67Ga reaction in the 5.9-8.7 MeV energy range using an activation technique. Natural Cu foils were bombarded with alpha beams from the 88 Cyclotron at Lawrence Berkeley National Laboratory (LBNL). Activated foils were counted using gamma spectrometry system at LBNL's Low Background Facility. The 63Cu(alpha,gamma)67Ga cross-sections were determined and compared with the latest NON-SMOKER theoretical values. Experimental cross sections were found to be in agreement with theoretical values.

  4. Recent developments in semiconductor gamma-ray detectors

    SciTech Connect

    Luke, Paul N.; Amman, Mark; Tindall, Craig; Lee, Julie S.

    2003-10-28

    The successful development of lithium-drifted Ge detectors in the 1960's marked the beginning of the significant use of semiconductor crystals for direct detection and spectroscopy of gamma rays. In the 1970's, high-purity Ge became available, which enabled the production of complex detectors and multi-detector systems. In the following decades, the technology of semiconductor gamma-ray detectors continued to advance, with significant developments not only in Ge detectors but also in Si detectors and room-temperature compound-semiconductor detectors. In recent years, our group at Lawrence Berkeley National Laboratory has developed a variety of gamma ray detectors based on these semiconductor materials. Examples include Ge strip detectors, lithium-drifted Si strip detectors, and coplanar-grid CdZnTe detectors. These advances provide new capabilities in the measurement of gamma rays, such as the ability to perform imaging and the realization of highly compact spectroscopy systems.

  5. Low radioactivity spectral gamma calibration facility

    SciTech Connect

    Mathews, M.A.; Bowman, H.R.; Huang, L., H.; Lavelle, M.J.; Smith, A.R.; Hearst, J.R.; Wollenberg, H.A.; Flexser, S.

    1986-01-01

    A low radioactivity calibration facility has been constructed at the Nevada Test Site (NTS). This facility has four calibration models of natural stone that are 3 ft in diameter and 6 ft long, with a 12 in. cored borehole in the center of each model and a lead-shielded run pipe below each model. These models have been analyzed by laboratory natural gamma ray spectroscopy (NGRS) and neutron activation analysis (NAA) for their K, U, and Th content. Also, 42 other elements were analyzed in the NAA. The /sup 222/Rn emanation data were collected. Calibrating the spectral gamma tool in this low radioactivity calibration facility allows the spectral gamma log to accurately aid in the recognition and mapping of subsurface stratigraphic units and alteration features associated with unusual concentrations of these radioactive elements, such as clay-rich zones.

  6. Rehabilitation of gamma

    NASA Astrophysics Data System (ADS)

    Poynton, Charles A.

    1998-07-01

    Gamma characterizes the reproduction of tone scale in an imaging system. Gamma summarizes, in a single numerical parameter, the nonlinear relationship between code value--in an 8-bit system, from 0 through 255--and physical intensity. Nearly all image coding systems are nonlinear, and so involve values of gamma different from unity. Owing to poor understanding of tone scale reproduction, and to misconceptions about nonlinear coding, gamma has acquired a terrible reputation in computer graphics and image processing. In addition, the world-wide web suffers from poor reproduction of grayscale and color images, due to poor handling of nonlinear image coding. This paper aims to make gamma respectable again.

  7. ESR response of gamma-irradiated sulfamethazine

    NASA Astrophysics Data System (ADS)

    Çolak, Seyda; Korkmaz, Mustafa

    In the present work, characteristic features of the radiolytical intermediates produced in gamma-irradiated solid sulfamethazine (SMH) were investigated by electron spin resonance (ESR) spectroscopy. The heights of the resonance peaks, measured with respect to the spectrum baseline, were used to monitor microwave saturation, temperature and time-dependent kinetic features of the radical species contributing to the formation of recorded experimental ESR spectra. Three species having different spectroscopic and kinetic features were observed to be produced in gamma-irradiated SMH. SO2, which is the most sensitive group of radiation in the SMH molecule, was found to be at the origin of radiation-produced ionic radical species. Based on the experimental results derived from the present study, the applicability of ESR spectroscopy to radiosterilization of SMH was discussed. In the dose range of interest (0.5-10 kGy), the radiation yield of solid SMH was calculated to be very low (G=0.45) compared with those obtained for sulfonamide aqueous solutions (G=3.5-5.1). Based on these findings, it was concluded that SMH and SMH-containing drugs could be safely sterilized by gamma radiation and that ESR spectroscopy could be successfully used as a potential technique for monitoring their radiosterilization.

  8. Modern Spectroscopy

    ERIC Educational Resources Information Center

    Barrow, Gordon M.

    1970-01-01

    Presents the basic ideas of modern spectroscopy. Both the angular momenta and wave-nature approaches to the determination of energy level patterns for atomic and molecular systems are discussed. The interpretation of spectra, based on atomic and molecular models, is considered. (LC)

  9. Space spectroscopy

    SciTech Connect

    Krupa, Tyler J.

    2000-02-01

    Los Alamos researchers have developed a technique to determine the composition of rock samples despite weather-induced mineral varnish deposited on the rocks. Using laser-induced breakdown spectroscopy (LIBS), the researchers determined the true elemental composition of a Mojave Desert rock sample with a thick weather-induced deposit on it. (AIP) (c)

  10. Isotopic composition analysis and age dating of uranium samples by high resolution gamma ray spectrometry

    NASA Astrophysics Data System (ADS)

    Apostol, A. I.; Pantelica, A.; Sima, O.; Fugaru, V.

    2016-09-01

    Non-destructive methods were applied to determine the isotopic composition and the time elapsed since last chemical purification of nine uranium samples. The applied methods are based on measuring gamma and X radiations of uranium samples by high resolution low energy gamma spectrometric system with planar high purity germanium detector and low background gamma spectrometric system with coaxial high purity germanium detector. The "Multigroup γ-ray Analysis Method for Uranium" (MGAU) code was used for the precise determination of samples' isotopic composition. The age of the samples was determined from the isotopic ratio 214Bi/234U. This ratio was calculated from the analyzed spectra of each uranium sample, using relative detection efficiency. Special attention is paid to the coincidence summing corrections that have to be taken into account when performing this type of analysis. In addition, an alternative approach for the age determination using full energy peak efficiencies obtained by Monte Carlo simulations with the GESPECOR code is described.

  11. The Gamma-Ray Imaging Spectrometer (GRIS): A new balloon-borne experiment for gamma-ray line astronomy

    NASA Technical Reports Server (NTRS)

    Teegarden, B. J.; Cline, T. L.; Gehrels, N.; Porreca, G.; Tueller, J.; Leventhal, M.; Huters, A. F.; Maccallum, C. J.; Stang, P. D.

    1985-01-01

    High resolution gamma-ray spectroscopy is a relatively new field that holds great promise for further understanding of high energy astrophysical processes. When the high resolution gamma-ray spectrometer (GRSE) was removed from the GRO payload, a balloon program was initiated to permit continued development and improvement of instrumentation in this field, as well as continued scientific observations. The Gamma-Ray Imaging Spectrometer (GRIS) is one of the experiments selected as part of this program. The instrument contains a number of new and innovative features that are expected to produce a significant improvement in source location accuracy and sensitivity over previous balloon and satellite experiments.

  12. New insights from cosmic gamma rays

    NASA Astrophysics Data System (ADS)

    Roland, Diehl

    2016-04-01

    The measurement of gamma rays from cosmic sources at ~MeV energies is one of the key tools for nuclear astrophysics, in its study of nuclear reactions and their impacts on objects and phenomena throughout the universe. Gamma rays trace nuclear processes most directly, as they originate from nuclear transitions following radioactive decays or high-energy collisions with excitation of nuclei. Additionally, the unique gamma-ray signature from the annihilation of positrons falls into this astronomical window and is discussed here: Cosmic positrons are often produced from β-decays, thus also of nuclear physics origins. The nuclear reactions leading to radioactive isotopes occur inside stars and stellar explosions, which therefore constitute the main objects of such studies. In recent years, both thermonuclear and core-collapse supernova radioactivities have been measured though 56Ni, 56Co, and 44Ti lines, and a beginning has thus been made to complement conventional supernova observations with such measurements of the prime energy sources of supernova light created in their deep interiors. The diffuse radioactive afterglow of massive-star nucleosynthesis in gamma rays is now being exploited towards astrophysical studies on how massive stars feed back their energy and ejecta into interstellar gas, as part of the cosmic cycle of matter through generations of stars enriching the interstellar gas and stars with metals. Large interstellar cavities and superbubbles have been recognised to be the dominating structures where new massive-star ejecta are injected, from 26Al gamma-ray spectroscopy. Also, constraints on the complex interiors of stars derive from the ratio of 60Fe/26Al gamma rays. Finally, the puzzling bulge-dominated intensity distribution of positron annihilation gamma rays is measured in greater detail, but still not understood; a recent microquasar flare provided evidence that such objects may be prime sources for positrons in interstellar space, rather than

  13. Spectroscopy of 215Rn86

    SciTech Connect

    Debray, M. E.; Davidson, M.; Davidson, J.; Hojman, D.; Kreiner, A. J.; Cardona, M. A.; Lenzi, S.; Napoli, D.

    2007-02-12

    The yrast level structure of 215,216Rn has been studied using in beam spectroscopy {alpha} - {gamma} - {gamma} coincidence techniques mainly through the 207Pb(18O, 2{alpha}2n) and 208Pb(18O, 2{alpha}2n) reactions in the 91-93 MeV energy range, using the 8{pi} GASP-ISIS spectrometer at Legnaro. The obtained low lying level scheme of 215Rn does not exhibit the alternating parity structure observed in their heavier known isotones 216Fr, 217Ra and 218Ac. The level scheme of 216Rn resulting from this study shows >From this result, the lightest nucleus showing evidence for reflection asymmetry is 216Fr defining one lowest-mass corner for this kind of phenomenon as N{>=}129 and Z{>=}87.

  14. Gamma ray transients

    NASA Technical Reports Server (NTRS)

    Cline, Thomas L.

    1987-01-01

    The discovery of cosmic gamma ray bursts was made with systems designed at Los Alamos Laboratory for the detection of nuclear explosions beyond the atmosphere. HELIOS-2 was the first gamma ray burst instrument launched; its initial results in 1976, seemed to deepen the mystery around gamma ray transients. Interplanetary spacecraft data were reviewed in terms of explaining the behavior and source of the transients.

  15. Gamma Oscillation in Schizophrenia

    PubMed Central

    O'Donnell, Brian F.; Youn, Soyoung; Kwon, Jun Soo

    2011-01-01

    Dysfunctional neural circuitry has been found to be involved in abnormalities of perception and cognition in patients with schizophrenia. Gamma oscillations are essential for integrating information within neural circuits and have therefore been associated with many perceptual and cognitive processes in healthy human subjects and animals. This review presents an overview of the neural basis of gamma oscillations and the abnormalities in the GABAergic interneuronal system thought to be responsible for gamma-range deficits in schizophrenia. We also review studies of gamma activity in sensory and cognitive processes, including auditory steady state response, attention, object representation, and working memory, in animals, healthy humans and patients with schizophrenia. PMID:22216037

  16. {gamma} production at CDF

    SciTech Connect

    Abe, F.

    1995-07-01

    We report on preliminary measurements of the {gamma}(1S), {gamma}(2S) and {gamma}(3S) differential and integrated cross sections in p{bar p} at {radical}s = 1.8 TeV using a sample of 16.6 {+-} 0.6 pb{sup -1} collected by the Collider Detector at Fermilab. The three resonances were reconstructed through the decay {gamma} {yields} {mu}{sup +}{mu}{sup -} in the rapidity region {vert_bar}y{vert_bar} < 0.4. The cross section results are compared to theoretical models of direct bottomonium production.

  17. Grain Spectroscopy

    NASA Technical Reports Server (NTRS)

    Allamandola, L. J.

    1992-01-01

    Our fundamental knowledge of interstellar grain composition has grown substantially during the past two decades thanks to significant advances in two areas: astronomical infrared spectroscopy and laboratory astrophysics. The opening of the mid-infrared, the spectral range from 4000-400 cm(sup -1) (2.5-25 microns), to spectroscopic study has been critical to this progress because spectroscopy in this region reveals more about a materials molecular composition and structure than any other physical property. Infrared spectra which are diagnostic of interstellar grain composition fall into two categories: absorption spectra of the dense and diffuse interstellar media, and emission spectra from UV-Vis rich dusty regions. The former will be presented in some detail, with the latter only very briefly mentioned. This paper summarized what we have learned from these spectra and presents 'doorway' references into the literature. Detailed reviews of many aspects of interstellar dust are given.

  18. Gamma-aminobutyric acid and glutamic acid levels in the auditory pathway of rats with chronic tinnitus: a direct determination using high resolution point-resolved proton magnetic resonance spectroscopy (1H-MRS)

    PubMed Central

    Brozoski, Thomas; Odintsov, Boris; Bauer, Carol

    2012-01-01

    Damage to the auditory system following high-level sound exposure reduces afferent input. Homeostatic mechanisms appear to compensate for the loss. Overcompensation may produce the sensation of sound without an objective physical correlate, i.e., tinnitus. Several potential compensatory neural processes have been identified, such as increased spontaneous activity. The cellular mechanisms enabling such compensatory processes may involve down-regulation of inhibitory neurotransmission mediated by γ-amino butyric acid (GABA), and/or up-regulation of excitatory neurotransmission, mediated by glutamic acid (Glu). Because central processing systems are integrated and well-regulated, compensatory changes in one system may produce reactive changes in others. Some or all may be relevant to tinnitus. To examine the roles of GABA and Glu in tinnitus, high resolution point-resolved proton magnetic resonance spectroscopy (1H-MRS) was used to quantify their levels in the dorsal cochlear nucleus (DCN), inferior colliculus (IC), medial geniculate body (MGB), and primary auditory cortex (A1) of rats. Chronic tinnitus was produced by a single high-level unilateral exposure to noise, and was measured using a psychophysical procedure sensitive to tinnitus. Decreased GABA levels were evident only in the MGB, with the greatest decrease, relative to unexposed controls, obtained in the contralateral MGB. Small GABA increases may have been present bilaterally in A1 and in the contralateral DCN. Although Glu levels showed considerable variation, Glu was moderately and bilaterally elevated both in the DCN and in A1. In the MGB Glu was increased ipsilaterally but decreased contralaterally. These bidirectional and region-specific alterations in GABA and Glu may reflect large-scale changes in inhibitory and excitatory equilibrium accompanying chronic tinnitus. The present results also suggest that targeting both neurotransmitter systems may be optimal in developing more effective therapeutics

  19. Raman spectroscopy

    SciTech Connect

    Gerrard, D.L.; Bowley, H.J.

    1986-04-01

    The period of this review is from late 1983 to late 1985. During this time over 5000 papers have appeared in the scientific literature dealing with many applications of Raman spectroscopy and extending its use to several new areas of study. As in the previous review in this series most of the applications relevant to solids are covered in one or other of the ten categories, which are the same as those used previously. However, aspects relating to solids which are not covered elsewhere include general reviews and the specific field of semiconductors. This is an area of great current interest in terms of Raman spectroscopy and the characterization of semiconductor materials and surfaces has been reported. Raman scattering also provides a new probe for the elucidation of structural properties of microcrystalline silicon and resonance Raman scattering in silicon at elevated temperatures has been studied. Many studies on carbon have also appeared in the literature including that of the various types of carbon, the use of Raman scattering to investigate disorder and crystallite formation in annealed carbon, in situ studies of intercalation kinetics, structural aspects of cokes and coals, and instrumentation for coal gasification. Raman spectroscopy has been applied to such diverse systems as organic crystals, the determination of modifications in layered crystals, the detection of explosives on silica gel or carbon, diagnostics of heterogeneous chemical processes, and a study of tungsten-halogen bulbs. Laser Raman spectroscopy has also been coupled with liquid chromatography and phase-resolved background suppression has been used to enhance Raman spectra. 397 references.

  20. Gamma detectors based on high-pressure xenon: their development and application

    NASA Astrophysics Data System (ADS)

    Ulin, Sergey E.; Dmitrenko, Valery V.; Grachev, V. M.; Uteshev, Z. M.; Vlasik, K. F.; Chernysheva, I. V.; Dukhvalov, A. G.; Kotler, F. G.; Pushkin, K. N.

    2004-10-01

    Various modifications of xenon detectors and their parameters in comparison with gamma-detectors of other types are considered. Prospects of xenon detectors' applicatins in gamma-spectroscopy based on experimental results are discussed including detection and control of radioactive and fissile materials displacement, definition of uranium enrichment rate, and measurements of nuclear reactor radioactive gas waste concentration. Possibilities for xenon detector use for environmental control and measurement of cosmic gamma radiation on orbital stations are considered.

  1. Gamma detectors based on high pressure xenon: their development and application

    NASA Astrophysics Data System (ADS)

    Ulin, Sergey E.; Dmitrenko, Valery V.; Grachev, V. M.; Uteshev, Z. M.; Vlasic, K. F.; Chernysheva, I. V.; Duhvalov, A. G.; Kotler, F. G.; Pushkin, K. N.

    2004-01-01

    Various modifications of xenon detectors and their parameters in comparison with gamma-detectors of other types are considered. Prospects of xenon detectors' applications in gamma-spectroscopy based on experimental results are discussed including detection and control of radioactive and fissile materials displacement, definition of uranium enrichment rate, and measurements of nuclear reactor radioactive gas waste concentration. Possibilities for xenon detector use for environmental control and measurement of cosmic gamma radiation on orbital stations are considered.

  2. Neutron-Capture Gamma-Ray Data for Obtaining Elemental Abundances from Planetary Spectra

    NASA Technical Reports Server (NTRS)

    Frankle, S. C.; Reedy, R. C.

    2001-01-01

    Newly compiled and evaluated energies and intensities of gamma rays made by the capture of thermal neutrons by elements from H to Zn plus Ge, Sm, and Gd are reported for use in determining elemental composition by planetary gamma-ray spectroscopy. Additional information is contained in the original extended abstract.

  3. Laser Spectroscopy

    NASA Astrophysics Data System (ADS)

    Katori, H.; Yoneda, H.; Nakagawa, K.; Shimizu, F.

    2010-02-01

    Anderson localization of matter-waves in a controlled disorder: a quantum simulator? / A. Aspect ... [et al.] -- Squeezing and entanglement in a Bose-Einstein condensate / C. Gross ... [et al.] -- New physics in dipolar Bose-Einstein condensates / Y. Kawaguchi, H. Saito, and M. Ueda -- Observation of vacuum fluctuations in a spinor Bose-Einstein condensate / C. Klempt ... [et al.] -- Negative-index media for matter waves / F. Perales ... [et al.] -- Entanglement of two individual atoms using the Rydberg blockade / A. Browaeys ... [et al.] -- Array of mesoscopic ensembles on a magnetic atom chip / A. F. Tauschinsky ... [et al.] -- Stability of the proton-to-electron mass ratio tested with molecules using an optical link to primary clock / A. Amy-Klein ... [et al.] -- Metastable helium: lifetime measurements using cold atoms as a test of QED / K. G. H. Baldwin ... [et al.] -- Optical lattice clocks with single occupancy bosons and spin-polarized fermions toward 10[symbol] accuracy / M. Takamoto ... [et al.] -- Frequency measurements of Al[symbol] and Hg[symbol] optical standards / W. M. Itano ... [et al.] -- Switching of light with light using cold atoms inside a hollow optical fiber / M. Bajcsy ... [et al.] -- Room-temperature atomic ensembles for quantum memory and magnetometry / K. Jensen ... [et al.] -- Components for multi-photon non-classical state preparation and measurement / G. Puentes ... [et al.] -- Quantum field state measurement and reconstruction in a cavity by quantum nondemolition photon counting / M. Brune ... [et al.] -- XUV frequency comb spectroscopy / C. Gohle ... [et al.] -- Ultrahigh-repetition-rate pulse train with absolute-phase control produced by an adiabatic raman process / M. Katsuragawa ... [et al.] -- Strongly correlated bosons and fermions in optical lattices / S. Will ... [et al.] -- Bragg spectroscopy of ultracold bose gases in optical lattices / L. Fallani ... [et al.] -- Synthetic quantum many-body systems / C. Guerlin ... [et al

  4. Muons in gamma showers

    NASA Technical Reports Server (NTRS)

    Stanev, T.; Vankov, C. P.; Halzen, F.

    1985-01-01

    Muon production in gamma-induced air showers, accounting for all major processes. For muon energies in the GeV region the photoproduction is by far the most important process, while the contribution of micron + micron pair creation is not negligible for TeV muons. The total rate of muons in gamma showers is, however, very low.

  5. Directional gamma detector

    DOEpatents

    LeVert, Francis E.; Cox, Samson A.

    1981-01-01

    An improved directional gamma radiation detector has a collector sandwiched etween two layers of insulation of varying thicknesses. The collector and insulation layers are contained within an evacuated casing, or emitter, which releases electrons upon exposure to gamma radiation. Delayed electrons and electrons entering the collector at oblique angles are attenuated as they pass through the insulation layers on route to the collector.

  6. Gamma-ray astrophysics

    NASA Technical Reports Server (NTRS)

    Stecker, F. W. (Editor); Trombka, J. I. (Editor)

    1973-01-01

    Conference papers on gamma ray astrophysics are summarized. Data cover the energy region from about 0.3 MeV to a few hundred GeV and theoretical models of production mechanisms that give rise to both galactic and extragalactic gamma rays.

  7. Optical gamma thermometer

    DOEpatents

    Koster, Glen Peter; Xia, Hua; Lee, Boon Kwee

    2013-08-06

    An optical gamma thermometer includes a metal mass having a temperature proportional to a gamma flux within a core of a nuclear reactor, and an optical fiber cable for measuring the temperature of the heated metal mass. The temperature of the heated mass may be measured by using one or more fiber grating structures and/or by using scattering techniques, such as Raman, Brillouin, and the like. The optical gamma thermometer may be used in conjunction with a conventional reactor heat balance to calibrate the local power range monitors over their useful in-service life. The optical gamma thermometer occupies much less space within the in-core instrument tube and costs much less than the conventional gamma thermometer.

  8. ESR identification of gamma-irradiated albendazole

    NASA Astrophysics Data System (ADS)

    Çolak, Seyda

    2010-01-01

    The use of ionizing radiation for sterilization of pharmaceuticals is a well-established technology. In the present work, the spectroscopic and kinetic features of the radicals induced in gamma-irradiated solid albendazole samples is investigated at different temperatures in the dose range of 3-34 kGy by electron spin resonance (ESR) spectroscopy. Irradiation with gamma radiation produced two different radical species in albendazole. They were fairly stable at room temperature but relatively unstable above room temperature, giving rise to an unresolved ESR spectrum consisting of three resonance peaks centered at g=2.0057. Decay activation energies of the contributing radical species were calculated to be 47.8 (±13.5) and 50.5 (±9.7) kJ/mol using the signal intensity decay data derived from annealing studies performed at high temperatures. A linear function of the applied dose was found to best describe the experimental dose-response data. Albendazole does not present the characteristics of good dosimetric materials. However, the discrimination of irradiated albendazole from its unirradiated form was possible even 6 months after storage in normal conditions. Based on these findings, it is concluded that albendazole and albendazole-containing drugs can be safely sterilized by gamma radiation and that ESR spectroscopy could be successfully used as a potential technique for monitoring their radiosterilization.

  9. Raman spectroscopy

    SciTech Connect

    Gerrard, D.L.; Bowley, H.J.

    1988-06-15

    The period of this review is from late 1985 to late 1987. During this time over 6000 papers have been published in the scientific literature dealing with many applications of Raman spectroscopy and extending its use to new areas of study. This article covers only those papers that are relevant to the analytical chemist and this necessitates a highly selective approach. There are some areas that have been the subject of many papers with relatively few being of analytical interest. In such cases the reader is referred to appropriate reviews which are detailed in this section.

  10. Hypernuclear spectroscopy

    SciTech Connect

    F. Garibaldi, O. Hashimoto, J.J. LeRose, P. Markowitz, S.N. Nakamura, J. Reinhold, L. Tang

    2011-06-01

    A program of hypernuclear spectroscopy experiments encompassing many hypernuclei has been undertaken in both Halls A and C using complimentary approaches. Spectra with sub-MeV resolution have been obtained for Li, B, and N in Hall A, while results from Hall C include He, B, and Al with new data still under analysis for He, Li, Be, B and V. High resolution and high precision in the determination of the single Λ binding energy at various shell levels has been the key success of these experiments using the (e,e'K+) reaction to produce Λ hypernuclei.

  11. Differential sensitivity of Chironomus and human hemoglobin to gamma radiation.

    PubMed

    Gaikwad, Pallavi S; Panicker, Lata; Mohole, Madhura; Sawant, Sangeeta; Mukhopadhyaya, Rita; Nath, Bimalendu B

    2016-08-01

    Chironomus ramosus is known to tolerate high doses of gamma radiation exposure. Larvae of this insect possess more than 95% of hemoglobin (Hb) in its circulatory hemolymph. This is a comparative study to see effect of gamma radiation on Hb of Chironomus and humans, two evolutionarily diverse organisms one having extracellular and the other intracellular Hb respectively. Stability and integrity of Chironomus and human Hb to gamma radiation was compared using biophysical techniques like Dynamic Light Scattering (DLS), UV-visible spectroscopy, fluorescence spectrometry and CD spectroscopy after exposure of whole larvae, larval hemolymph, human peripheral blood, purified Chironomus and human Hb. Sequence- and structure-based bioinformatics methods were used to analyze the sequence and structural similarities or differences in the heme pockets of respective Hbs. Resistivity of Chironomus Hb to gamma radiation is remarkably higher than human Hb. Human Hb exhibited loss of heme iron at a relatively low dose of gamma radiation exposure as compared to Chironomus Hb. Unlike human Hb, the heme pocket of Chironomus Hb is rich in aromatic amino acids. Higher hydophobicity around heme pocket confers stability of Chironomus Hb compared to human Hb. Previously reported gamma radiation tolerance of Chironomus can be largely attributed to its evolutionarily ancient form of extracellular Hb as evident from the present study. PMID:27237970

  12. Pulser injection with subsequent removal for gamma-ray spectrometry

    DOEpatents

    Hartwell, Jack K.; Goodwin, Scott G.; Johnson, Larry O.; Killian, E. Wayne

    1990-01-01

    An improved system for gamma-ray spectroscopy characterized by an interface module that controls the injection of electronic pulses as well as separation logic that enables storage of pulser events in a region of the spectrum of a multichannel analyzer distinct from the region reserved for storage of gamma-ray events. The module accomplishes this by tagging pulser events (high or low) injected into the amplification circuitry, adding an offset to the events so identified at the time the events are at the output of the analog to digital converter, and storing such events in the upper portion of the spectrum stored in the multichannel analyzer. The module can be adapted for use with existing gamma-ray spectroscopy equipment to provide for automatic analyses of radioisotopes.

  13. Attosecond Spectroscopy

    NASA Astrophysics Data System (ADS)

    Schultze, Martin

    2011-05-01

    Attosecond spectroscopy is enabled by the advent of intense ultrashort light pulses comprising merely a few wave cycles. Manipulating the hyperfast-varying electric field evolution of these pulses permits the manipulation and tracking of the atomic-scale motion of electrons. A striking implication of this ability is the generation and characterization of isolated attosecond pulses of extreme ultraviolet (XUV) light and their characterization. Spectroscopic techniques making use of the unprecedented temporal resolution that attosecond XUV pulses offer can track and control electron dynamics in the interior of atoms, molecules as well as in solids and provide insight in the evolution of ultrafast electronic population dynamics and related coherent processes. Attosecond technology in combination with conventional electron spectroscopy, dubbed ``attosecond streaking'' investigates the timing of photoemission and electronic transport processes on solid surfaces. The extension of transient absorption measurement schemes makes coherent electronic dynamics accessible and the effects that ultrastrong and -short laser electric fields exert on the electronic structure of matter and the band structure population dynamics.

  14. Effect of gamma irradiation on DC electrical conductivity of ZnO nanoparticles

    SciTech Connect

    Swaroop, K.; Somashekarappa, H. M.; Naveen, C. S.; Jayanna, H. S.

    2015-06-24

    The temperature dependent dc electrical conductivity of gamma irradiated Zinc oxide (ZnO) nanoparticles is presented in this paper. The X-ray diffraction (XRD) pattern shows hexagonal wurtzite structure of ZnO. Fourier Transform Infrared Spectroscopy (FTIR) confirms Zn-O stretching vibrations. UV-Visible spectroscopy studies show that the energy band gap (E{sub g}) of the prepared ZnO nanoparticles increases with respect to gamma irradiation dose, which can be related to room temperature dc electrical conductivity. The result shows significant variation in the high temperature dc electrical conductivity of ZnO nanoparticles due to gamma irradiation.

  15. LASER-PLASMA-ACCELERATOR-BASED GAMMA GAMMA COLLIDERS

    SciTech Connect

    Schroeder, C. B.; Esarey, E.; Toth, Cs.; Geddes, C. G. R.; Leemans, W. P.

    2009-05-04

    Design considerations for a next-generation linear collider based on laser-plasma-accelerators are discussed, and a laser-plasma-accelerator-based gamma-gamma collider is considered. An example of the parameters for a 0.5 TeV laser-plasma-accelerator gamma gamma collider is presented.

  16. Resting GABA and glutamate concentrations do not predict visual gamma frequency or amplitude.

    PubMed

    Cousijn, Helena; Haegens, Saskia; Wallis, George; Near, Jamie; Stokes, Mark G; Harrison, Paul J; Nobre, Anna C

    2014-06-24

    Gamma band oscillations arise in neuronal networks of interconnected GABAergic interneurons and excitatory pyramidal cells. A previous study found a correlation between visual gamma peak frequency, as measured with magnetoencephalography, and resting GABA levels, as measured with magnetic resonance spectroscopy (MRS), in 12 healthy volunteers. If true, this would allow studies in clinical populations testing modulation of this relationship, but this finding has not been replicated. We addressed this important question by measuring gamma oscillations and GABA, as well as glutamate, in 50 healthy volunteers. Visual gamma activity was evoked using an established gratings paradigm, and we applied a beamformer spatial filtering technique to extract source-reconstructed gamma peak frequency and amplitude from the occipital lobe. We determined gamma peak frequency and amplitude from the location with maximal activation and from the location of the MRS voxel to assess the relationship of GABA with gamma. Gamma peak frequency was estimated from the highest value of the raw spectra and by a Gaussian fit to the spectra. MRS data were acquired from occipital cortex. We did not replicate the previously found correlation between gamma peak frequency and GABA concentration. Calculation of a Bayes factor provided strong evidence in favor of the null hypothesis. We also did not find a correlation between gamma activity and glutamate or between gamma and the ratio of GABA/glutamate. Our results suggest that cortical gamma oscillations do not have a consistent, demonstrable relationship to excitatory/inhibitory network activity as proxied by MRS measurements of GABA and glutamate. PMID:24927588

  17. Resting GABA and glutamate concentrations do not predict visual gamma frequency or amplitude

    PubMed Central

    Cousijn, Helena; Haegens, Saskia; Wallis, George; Near, Jamie; Stokes, Mark G.; Harrison, Paul J.; Nobre, Anna C.

    2014-01-01

    Gamma band oscillations arise in neuronal networks of interconnected GABAergic interneurons and excitatory pyramidal cells. A previous study found a correlation between visual gamma peak frequency, as measured with magnetoencephalography, and resting GABA levels, as measured with magnetic resonance spectroscopy (MRS), in 12 healthy volunteers. If true, this would allow studies in clinical populations testing modulation of this relationship, but this finding has not been replicated. We addressed this important question by measuring gamma oscillations and GABA, as well as glutamate, in 50 healthy volunteers. Visual gamma activity was evoked using an established gratings paradigm, and we applied a beamformer spatial filtering technique to extract source-reconstructed gamma peak frequency and amplitude from the occipital lobe. We determined gamma peak frequency and amplitude from the location with maximal activation and from the location of the MRS voxel to assess the relationship of GABA with gamma. Gamma peak frequency was estimated from the highest value of the raw spectra and by a Gaussian fit to the spectra. MRS data were acquired from occipital cortex. We did not replicate the previously found correlation between gamma peak frequency and GABA concentration. Calculation of a Bayes factor provided strong evidence in favor of the null hypothesis. We also did not find a correlation between gamma activity and glutamate or between gamma and the ratio of GABA/glutamate. Our results suggest that cortical gamma oscillations do not have a consistent, demonstrable relationship to excitatory/inhibitory network activity as proxied by MRS measurements of GABA and glutamate. PMID:24927588

  18. Fermi GBM Observations of Terrestrial Gamma Flashes

    NASA Technical Reports Server (NTRS)

    Wilson-Hodge, Colleen A.; Briggs, M. S.; Fishman, G. J.; Bhat, P. N.; Paciesas, W. S.; Preece, R.; Kippen, R. M.; von Kienlin, A.; Dwyer, J. R.; Smith, D. M.; Holzworth, R.

    2010-01-01

    In its first two years of operation, the Fermi Gamma Ray Burst Monitor (GBM) has observed more than 77 Terrestrial Gamma Flashes (TGFs). The thick Bismuth Germanate (BGO) detectors are excellent for TGF spectroscopy, having a high probability of recording the full energy of an incident photon, spanning a broad energy range from 150 keV to 40 MeV, and recording a large number of photons per TGF. Correlations between GBM TGF triggers and lightning sferics detected with the World-Wide Lightning Location Network indicate that TGFs and lightning are simultaneous to within tens of microseconds. The energy spectra of some TGFs have strong 511 keV positron annihilation lines, indicating that these TGFs contain a large fraction of positrons

  19. Prospects for gamma ray astronomy

    NASA Technical Reports Server (NTRS)

    1981-01-01

    The Solar Maximum Mission and the Gamma Ray Experiment aboard the SMM spacecraft are discussed. Mission plans for interplanetary probes are also discussed. The Gamma Ray observatory and its role in future gamma ray astronomy is highlighted. It is concluded that gamma ray astronomy will be of major importance in the development of astronomical models and in the development of comsological theory.

  20. THE {gamma}SF METHOD

    SciTech Connect

    Utsunomiya, H.; Akimune, H.; Yamagata, T.; Kondo, T.; Iwamoto, C.; Okamoto, A.; Goriely, S.; Harada, H.; Kitatani, F.; Goko, S.; Toyokawa, H.; Yamada, K.; Lui, Y.-W.; Hilaire, S.; Koning, A. J.

    2011-10-28

    The {gamma}-ray strength function ({gamma}SF) interconnects radiative neutron capture and photoneutron emission as a common ingredient in the statistical model. Outlined here is an indirect method of determining radiative neutron-capture cross sections for unstable nuclei based on the {gamma}-ray strength function. Application examples of the {gamma}SF method are demonstrated.

  1. The gamma-ray observatory

    NASA Technical Reports Server (NTRS)

    1991-01-01

    An overview is given of the Gamma Ray Observatory (GRO) mission. Detection of gamma rays and gamma ray sources, operations using the Space Shuttle, and instruments aboard the GRO, including the Burst and Transient Source Experiment (BATSE), the Oriented Scintillation Spectrometer Experiment (OSSE), the Imaging Compton Telescope (COMPTEL), and the Energetic Gamma Ray Experiment Telescope (EGRET) are among the topics surveyed.

  2. Gamma ray astronomy

    NASA Technical Reports Server (NTRS)

    Paciesas, William S.

    1991-01-01

    Miscellaneous tasks related to the development of the Bursts and Transient Source Experiment on the Gamma Ray Observatory and to analysis of archival data from balloon flight experiments were performed. The results are summarized and relevant references are included.

  3. Gamma-ray astronomy

    NASA Technical Reports Server (NTRS)

    Ramaty, R.; Lingenfelter, R. E.

    1982-01-01

    Cosmic gamma rays, the physical processes responsible for their production and the astrophysical sites from which they were seen are reported. The bulk of the observed gamma ray emission is in the photon energy range from about 0.1 MeV to 1 GeV, where observations are carried out above the atmosphere. There are also, however, gamma ray observations at higher energies obtained by detecting the Cerenkov light produced by the high energy photons in the atmosphere. Gamma ray emission was observed from sources as close as the Sun and the Moon and as distant as the quasar 3C273, as well as from various other galactic and extragalactic sites. The radiation processes also range from the well understood, e.g. energetic particle interactions with matter, to the still incompletely researched, such as radiation transfer in optically thick electron positron plasmas in intense neutron star magnetic fields.

  4. Gamma ray line astronomy

    NASA Technical Reports Server (NTRS)

    Ramaty, R.

    1984-01-01

    The interpretations and implications of the astrophysical observations of gamma-ray lines are reviewed. At the Galactic Center e(+)-e(-) pairs from a compact object produce an annihilation line that shows no redshift, indicating an annihilation site far removed from this object. In the jets of SS433, gamma-ray lines are produced by inelastic excitations, probably in dust grains, although line emission from fusion reactions has also been considered. Observations of diffuse galactic line emission reveal recently synthesized radioactive aluminum in the interstellar medium. In gamma-ray bursts, redshifted pair annihilation lines are consistent with a neutron star origin for the bursts. In solar flares, gamma-ray line emission reveals the prompt acceleration of protons and nuclei, in close association with the flare energy release mechanism.

  5. Gamma Ray Pulsars: Observations

    NASA Technical Reports Server (NTRS)

    Thompson, David J.; White, Nicholas E. (Technical Monitor)

    2000-01-01

    High-energy gamma rays are a valuable tool for studying particle acceleration and radiation in the magnetospheres of energetic pulsars. The six or more pulsars seen by CGRO/EGRET show that: the light curves usually have double-peak structures (suggesting a broad cone of emission); gamma rays are frequently the dominant component of the radiated power; and all the spectra show evidence of a high-energy turnover. Unless a new pulsed component appears at higher energies, progress in gamma-ray pulsar studies will be greatest in the 1-20 GeV range. Ground-based telescopes whose energy ranges extend downward toward 10 GeV should make important measurements of the spectral cutoffs. The Gamma-ray Large Area Space Telescope (GLAST), now in planning for a launch in 2005, will provide a major advance in sensitivity, energy range, and sky coverage.

  6. Dynamic gamma knife radiosurgery

    NASA Astrophysics Data System (ADS)

    Luan, Shuang; Swanson, Nathan; Chen, Zhe; Ma, Lijun

    2009-03-01

    Gamma knife has been the treatment of choice for various brain tumors and functional disorders. Current gamma knife radiosurgery is planned in a 'ball-packing' approach and delivered in a 'step-and-shoot' manner, i.e. it aims to 'pack' the different sized spherical high-dose volumes (called 'shots') into a tumor volume. We have developed a dynamic scheme for gamma knife radiosurgery based on the concept of 'dose-painting' to take advantage of the new robotic patient positioning system on the latest Gamma Knife C™ and Perfexion™ units. In our scheme, the spherical high dose volume created by the gamma knife unit will be viewed as a 3D spherical 'paintbrush', and treatment planning reduces to finding the best route of this 'paintbrush' to 'paint' a 3D tumor volume. Under our dose-painting concept, gamma knife radiosurgery becomes dynamic, where the patient moves continuously under the robotic positioning system. We have implemented a fully automatic dynamic gamma knife radiosurgery treatment planning system, where the inverse planning problem is solved as a traveling salesman problem combined with constrained least-square optimizations. We have also carried out experimental studies of dynamic gamma knife radiosurgery and showed the following. (1) Dynamic gamma knife radiosurgery is ideally suited for fully automatic inverse planning, where high quality radiosurgery plans can be obtained in minutes of computation. (2) Dynamic radiosurgery plans are more conformal than step-and-shoot plans and can maintain a steep dose gradient (around 13% per mm) between the target tumor volume and the surrounding critical structures. (3) It is possible to prescribe multiple isodose lines with dynamic gamma knife radiosurgery, so that the treatment can cover the periphery of the target volume while escalating the dose for high tumor burden regions. (4) With dynamic gamma knife radiosurgery, one can obtain a family of plans representing a tradeoff between the delivery time and the

  7. Raman Spectroscopy of Irradiated Tissue Samples

    NASA Astrophysics Data System (ADS)

    Alexa, P.; Synytsya, A.; Volka, K.; de Boer, J.; Besserer, J.; Froschauer, S.; Loewe, M.; Moosburger, M.; Würkner, M.

    2003-06-01

    Tissue samples (skin of mice, normal and tumor, skin of a woman, normal and tumor) were irradiated by protons from the Munich tandem accelerator. The samples were analysed using Raman spectroscopy at the Institute of Chemical Technology in Prague by measuring the intensity of signals sensitive to radiation damage. Effects depending on the delivered dose were found. Proton-irradiation effects are then compared to those of gamma-irradiation.

  8. Point contact spectroscopy of heavy fermions

    NASA Astrophysics Data System (ADS)

    Moser, M.; Wachter, P.; Franse, J. J. M.; Meisner, G. P.; Walker, E.

    Point contact spectroscopy (PCS) has been performed on the heavy fermion systems CeAl3, CeCu6, UPt3, U6Co and U2PtC2. The dynamical resistance dU/dI is a function of the electronic density of states (EDS) at E/sub F/. The width of the EDS inferred from the PC measurements can be compared with the (GAMMA)-value of the specific heat.

  9. Gamma-ray luminosity and photon index evolution of FSRQ blazars and contribution to the gamma-ray background

    SciTech Connect

    Singal, J.; Ko, A.; Petrosian, V.

    2014-05-10

    We present the redshift evolutions and distributions of the gamma-ray luminosity and photon spectral index of flat spectrum radio quasar (FSRQ) type blazars, using non-parametric methods to obtain the evolutions and distributions directly from the data. The sample we use for analysis consists of almost all FSRQs observed with a greater than approximately 7σ detection threshold in the first-year catalog of the Fermi Gamma-ray Space Telescope's Large Area Telescope, with redshifts as determined from optical spectroscopy by Shaw et al. We find that FSQRs undergo rapid gamma-ray luminosity evolution, but negligible photon index evolution, with redshift. With these evolutions accounted for we determine the density evolution and luminosity function of FSRQs and calculate their total contribution to the extragalactic gamma-ray background radiation, resolved and unresolved, which is found to be 16(+10/–4)%, in agreement with previous studies.

  10. Gamma ray camera

    SciTech Connect

    Robbins, C.D.; Wang, S.

    1980-09-09

    An anger gamma ray camera is improved by the substitution of a gamma ray sensitive, proximity type image intensifier tube for the scintillator screen in the anger camera, the image intensifier tube having a negatively charged flat scintillator screen and a flat photocathode layer and a grounded, flat output phosphor display screen all of the same dimension (Unity image magnification) and all within a grounded metallic tube envelope and having a metallic, inwardly concaved input window between the scintillator screen and the collimator.

  11. Monitoring Neutron Generator Output in a Mixed Neutron-Gamma Field Using a Plastic Scintillator.

    SciTech Connect

    Mitra,S.; Wielopolski, L.

    2007-10-28

    Quantitative neutron-induced gamma-ray spectroscopy employing neutron generators (NGs) entails monitoring them for possible fluctuations in their neutron output. We accomplished this using a plastic scintillator and recording a spectrum from which we selected a neutron region-of-interest (nROI) to discriminate between neutrons and the accompanying high-energy gamma-rays. We show that the selected nROI is insensitive to changes in the gamma-ray background, thus allowing satisfactory normalization of the gamma-ray spectra of an in-situ system for analyzing soil carbon.

  12. Design of a compact spectrometer for high-flux MeV gamma-ray beams

    SciTech Connect

    Corvan, D. J. Sarri, G.; Zepf, M.

    2014-06-15

    A novel design for a compact gamma-ray spectrometer is presented. The proposed system allows for spectroscopy of high-flux multi-MeV gamma-ray beams with MeV energy resolution in a compact design. In its basic configuration, the spectrometer exploits conversion of gamma-rays into electrons via Compton scattering in a low-Z material. The scattered electron population is then spectrally resolved using a magnetic spectrometer. The detector is shown to be effective for gamma-ray energies between 3 and 20 MeV. The main properties of the spectrometer are confirmed by Monte Carlo simulations.

  13. Gamma ray optics

    SciTech Connect

    Jentschel, M.; Guenther, M. M.; Habs, D.; Thirolf, P. G.

    2012-07-09

    Via refractive or diffractive scattering one can shape {gamma} ray beams in terms of beam divergence, spot size and monochromaticity. These concepts might be particular important in combination with future highly brilliant gamma ray sources and might push the sensibility of planned experiments by several orders of magnitude. We will demonstrate the experimental feasibility of gamma ray monochromatization on a ppm level and the creation of a gamma ray beam with nanoradian divergence. The results are obtained using the inpile target position of the High Flux Reactor of the ILL Grenoble and the crystal spectrometer GAMS. Since the refractive index is believed to vanish to zero with 1/E{sup 2}, the concept of refractive optics has never been considered for gamma rays. The combination of refractive optics with monochromator crystals is proposed to be a promising design. Using the crystal spectrometer GAMS, we have measured for the first time the refractive index at energies in the energy range of 180 - 2000 keV. The results indicate a deviation from simple 1/E{sup 2} extrapolation of X-ray results towards higher energies. A first interpretation of these new results will be presented. We will discuss the consequences of these results on the construction of refractive optics such as lenses or refracting prisms for gamma rays and their combination with single crystal monochromators.

  14. Instrument Requirements for Type Ia Supernova Gamma-Ray Studies

    NASA Astrophysics Data System (ADS)

    Leising, M.; Milne, P.; Lara, J.; The, L.

    2004-12-01

    Thermonuclear supernovae are widely used as distance indicators, which yields profound implications, yet details of their progenitor systems and explosion physics remain elusive. It has been argued for thirty-five years that these thoroughly radioactive objects can be understood through detailed gamma-ray line studies, but despite twenty years of gamma-ray instruments in orbit, no Type Ia supernova (SN Ia) has been detected in gamma-ray lines. Still the great promise of gamma-ray studies of SN Ia remains, but the instrument requirements, especially on line sensitivity, are substantial. Finally, a second-generation gamma-ray spectrometer, known now as the Advanced Compton Telescope, is being planned. Considering current SN Ia models of various types, including deflagrations, delayed detonations, and sub-Chandrasekhar-mass detonations, we outline the gamma-ray instrument requirements, especially line flux sensitivity and energy resolution, needed to discriminate among the possible models. We consider realistic SN Ia rates and distributions in space, plausible observing intervals and durations, and the information available from both gamma-ray photometry and spectroscopy. For example, we find that a wide-field compton telescope with energy resolution E/Δ E= 100 in a scanning mode would require broad line sensitivity of 7×10-7 cm-2 s-1 at 847 keV to distinguish deflagration models from delayed detonation models at the rate of one per year.

  15. Measurement of the {sup 241}Am({gamma},n){sup 240}Am reaction in the giant dipole resonance region

    SciTech Connect

    Tonchev, A. P.; Howell, C. R.; Hutcheson, A.; Kwan, E.; Raut, R.; Rusev, G.; Tornow, W.; Hammond, S. L.; Huibregtse, C.; Kelley, J. H.; Kawano, T.; Vieira, D. J.; Wilhelmy, J. B.

    2010-11-15

    The photodisintegration cross section of the radioactive nucleus {sup 241}Am has been obtained using activation techniques and monoenergetic {gamma}-ray beams from the HI{gamma}S facility. The induced activity of {sup 240}Am produced via the {sup 241}Am({gamma},n) reaction was measured in the energy interval from 9 to 16 MeV utilizing high-resolution {gamma}-ray spectroscopy. The experimental data for the {sup 241}Am({gamma},n) reaction in the giant dipole resonance energy region are compared with statistical nuclear-model calculations.

  16. Polycrystalline gamma plutonium's elastic moduli versus temperature

    SciTech Connect

    Migliori, Albert; Betts, J; Trugman, A; Mielke, C H; Mitchell, J N; Ramos, M; Stroe, I

    2009-01-01

    Resonant ultrasound spectroscopy was used to measure the elastic properties of pure polycrystalline {sup 239}Pu in the {gamma} phase. Shear and longitudinal elastic moduli were measured simultaneously and the bulk modulus was computed from them. A smooth, linear, and large decrease of all elastic moduli with increasing temperature was observed. They calculated the Poisson ratio and found that it increases from 0.242 at 519 K to 0.252 at 571 K. These measurements on extremely well characterized pure Pu are in agreement with other reported results where overlap occurs.

  17. Amateur spectroscopy

    NASA Astrophysics Data System (ADS)

    Gavin, M. V.

    1998-06-01

    (The 1997 Presidential Address to the British Astronomical Association.) Auguste Comte is remembered for an unfortunate remark. In 1825 he said the chemical composition of stars would never be revealed. Within a decade or so the heart of the atom was being explored in remote stars through the science of spectroscopy. In simplistic terms one can regard the atom as a miniature solar system, but with the novel option that electrons (representing planets) having the ability to 'jump' from one orbit to another. In 'falling' to a lower orbit a photon of light of precise wavelength is released to travel outwards. When the electron 'jumps' to a higher orbit a photon of light is absorbed. This is taking place on a vast scale which we observe as lines in the spectrum - their position and prominence relates to the particular atomic element, temperature and pressure within the stellar atmosphere. It is beyond the scope of this Address to discuss the various processes that affect spectra, or to provide a mathematical explanation which can be found elsewhere. In any case the lack of a deep understanding does not preclude enjoyable or useful observations. Methods and results from amateurs conducting such observations are discussed in this paper.

  18. MHD Spectroscopy

    SciTech Connect

    Heeter, R F; Fasoli, A; Testa, D; Sharapov, S; Berk, H L; Breizman, B; Gondhalekar, A; Mantsinen, M

    2004-03-23

    Experiments are conducted on the JET tokamak to assess the diagnostic potential of MHD active and passive spectroscopy, for the plasma bulk and its suprathermal components, using Alfv{acute e}n Eigenmodes (AEs) excited by external antennas and by energetic particles. The measurements of AE frequencies and mode numbers give information on the bulk plasma. Improved equilibrium reconstruction, in particular in terms of radial profiles of density and safety factor, is possible from the comparison between the antenna driven spectrum and that calculated theoretically. Details of the time evolution of the non-monotonic safety factor profile in advanced scenarios can be reconstructed from the frequency of ICRH-driven energetic particle modes. The plasma effective mass can be inferred from the resonant frequency of externally driven AEs in discharges with similar equilibrium profiles. The stability thresholds and the nonlinear development of the instabilities can give clues on energy and spatial distribution of the fast particle population. The presence of unstable AEs provides lower limits in the energy of ICRH generated fast ion tails. Fast ion pressure gradients and their evolution can be inferred from the stability of AEs at different plasma radial positions. Finally, the details of the AE spectrum in the nonlinear stage can be used to obtain information about the fast particle velocity space diffusion.

  19. Planetary spectroscopy

    NASA Technical Reports Server (NTRS)

    Fink, Uwe

    1988-01-01

    The main goal of the research is charge coupled device (CCD) spectroscopic and imaging studies of the solar system in support of spacecraft investigations. Studies include the physical behavior of comets, the atmosphere of the gaseous planets, and the solid surfaces of satellites and asteroids. The major observing program consisted of approximately 50 nights of photometry of Comet Halley in order to resolve the controversy over this comet's rotation period. This data is presently being analyzed. Additional observing projects included the spectroscopic occultation of Charon by Pluto, reflection spectroscopy of Mercury, and a spectrum of the satellite Oberon. Mercury data does not corroborate the Fe(++) absorption feature reported by McCord and Clark at 8800 A but instead potentially shows a weaker feature at longer wavelengths. This position is in much closer accord with expectations for Mercury since a band center near 8800 A implies too little Fe(++) on Mercury, especially if band shifts with temperature are considered. The Pluto project proved that the deep methane absorptions visible in their combined specta are due soley to Pluto with Charon showing a flat and featureless spectrum. It appears that if Charon ever contained a substantial methane component, the satellite's low surface gravity could not hold it and the methane evaporated and escaped.

  20. SIMP spectroscopy

    NASA Astrophysics Data System (ADS)

    Hochberg, Yonit; Kuflik, Eric; Murayama, Hitoshi

    2016-05-01

    We study the interactions between strongly interacting massive particle dark matter and the Standard Model via a massive vector boson that is kinetically mixed with the hypercharge gauge boson. The relic abundance is set by 3 → 2 self-interactions of the dark matter, while the interactions with the vector mediator enable kinetic equilibrium between the dark and visible sectors. We show that a wide range of parameters is phenomenologically viable and can be probed in various ways. Astrophysical and cosmological constraints are evaded due to the p-wave nature of dark matter annihilation into visible particles, while direct detection methods using electron recoils can be sensitive to parts of the parameter space. In addition, we propose performing spectroscopy of the strongly coupled dark sector at e + e - colliders, where the energy of a mono-photon can track the resonance structure of the dark sector. Alternatively, some resonances may decay back into Standard Model leptons or jets, realizing `hidden valley' phenomenology at the LHC and ILC in a concrete fashion.