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Sample records for magnetic anisotropy field

  1. Anisotropy in MHD turbulence due to a mean magnetic field

    NASA Technical Reports Server (NTRS)

    Shebalin, J. V.; Matthaeus, W. H.; Montgomery, D.

    1982-01-01

    The development of anisotropy in an initially isotropic spectrum is studied numerically for two-dimensional magnetohydrodynamic turbulence. The anisotropy develops due to the combined effects of an externally imposed dc magnetic field and viscous and resistive dissipation at high wave numbers. The effect is most pronounced at high mechanical and magnetic Reynolds numbers. The anisotropy is greater at the higher wave numbers.

  2. Electric field controlled magnetic anisotropy in a single molecule.

    PubMed

    Zyazin, Alexander S; van den Berg, Johan W G; Osorio, Edgar A; van der Zant, Herre S J; Konstantinidis, Nikolaos P; Leijnse, Martin; Wegewijs, Maarten R; May, Falk; Hofstetter, Walter; Danieli, Chiara; Cornia, Andrea

    2010-09-01

    We have measured quantum transport through an individual Fe(4) single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are observed in inelastic tunneling spectroscopy. We demonstrate that the molecule retains its magnetic properties and, moreover, that the magnetic anisotropy is significantly enhanced by reversible electron addition/subtraction controlled with the gate voltage. Single-molecule magnetism can thus be electrically controlled. PMID:20687519

  3. Electric Field Controlled Magnetic Anisotropy in a Single Molecule

    NASA Astrophysics Data System (ADS)

    Zyazin, Alexander S.; van den Berg, Johan W. G.; Osorio, Edgar A.; van der Zant, Herre S. J.; Konstantinidis, Nikolaos P.; Leijnse, Martin; Wegewijs, Maarten R.; May, Falk; Hofstetter, Walter; Danieli, Chiara; Cornia, Andrea

    2010-09-01

    We have measured quantum transport through an individual Fe$_4$ single-molecule magnet embedded in a three-terminal device geometry. The characteristic zero-field splittings of adjacent charge states and their magnetic field evolution are observed in inelastic tunneling spectroscopy. We demonstrate that the molecule retains its magnetic properties, and moreover, that the magnetic anisotropy is significantly enhanced by reversible electron addition / subtraction controlled with the gate voltage. Single-molecule magnetism can thus be electrically controlled.

  4. Magnetic stress anisotropy field in plated cylindrical Permalloy films.

    NASA Technical Reports Server (NTRS)

    Lutes, O. S.

    1971-01-01

    An analysis is made of the magnetic stress anisotropy field (Hks) arising from internal and external stress sources in plated-wire memory elements. The analysis takes into consideration circumferential composition variation and cylindrical geometry of the Permalloy film. Expressions are derived relating Hks to uniaxial film stress, average composition, and amplitude of composition variation. A result of particular importance is that even for average zeromagnetostrictive composition (ZMC) films, Hks may still make an appreciable contribution to the total anisotropy field if the composition is not uniform. Calculated Hks characteristics are shown to correlate with anisotropy field changes observed in annealing experiments. Examples are given to show the importance of composition uniformity in determining the stability of the anisotropy field. The utility of the analysis is extended by the inclusion of data expressing the inverse relation between anisotropy field and easy-axis dispersion in the film.

  5. Enhanced cosmic ray anisotropies and the extended solar magnetic field

    SciTech Connect

    Swinson, D.B.; Saito, T.; Mori, S.

    1981-10-01

    Saito's two-hemisphere model for the three-dimensional magnetic structure of the inner heliomagnetosphere is used to determine the orientation of the two solar magnetic hemispheres. This orientation, as viewed from the earth, varies throughout the year. The orientations during 1974 are presented and are confirmed by satellite data for the interplanetary magnetic field. These data suggest a role for the field component perpendicular to the ecliptic plane B/sub z/ in giving rise to cosmic ray anisotropies detected at the earth. It is shown that an enhanced solar diurnal variation in cosmic ray intensity at the earth can arise from the constructive interference of three cosmic ray anisotropies, two of which depend on the direction of the interplanetary magnetic field. This is demonstrated by using cosmic ray data from the Nagaya muon telescope and underground muon telescopes in Bolivia, Embudo (New Mexico), and Socorro (New Mexico).

  6. Anisotropy of photon production: initial eccentricity or magnetic field.

    PubMed

    Bzdak, Adam; Skokov, Vladimir

    2013-05-10

    Recent measurements of the azimuthal anisotropy of direct photons in heavy-ion collisions at the energies of Relativistic Heavy Ion Collider show that it is of the same order as the hadronic one. This finding appears to contradict the expected dominance of photon production from a quark-gluon plasma at an early stage of a heavy-ion collision. A possible explanation of the strong azimuthal anisotropy of the photons, given recently, is based on the presence of a large magnetic field in the early phase of a collision. In this Letter, we propose a method to experimentally measure the degree to which a magnetic field in heavy-ion collisions is responsible for the observed anisotropy of photon production. The experimental test proposed in this Letter may potentially change our understanding of the nonequilibrium stage and possible thermalization in heavy-ion collisions. PMID:23705700

  7. Anisotropies in magnetic field evolution and local Lyapunov exponents

    SciTech Connect

    Tang, X.Z.; Boozer, A.H.

    2000-01-13

    The natural occurrence of small scale structures and the extreme anisotropy in the evolution of a magnetic field embedded in a conducting flow is interpreted in terms of the properties of the local Lyapunov exponents along the various local characteristic (un)stable directions for the Lagrangian flow trajectories. The local Lyapunov exponents and the characteristic directions are functions of Lagrangian coordinates and time, which are completely determined once the flow field is specified. The characteristic directions that are associated with the spatial anisotropy of the problem, are prescribed in both Lagrangian and Eulerian frames. Coordinate transformation techniques are employed to relate the spatial distributions of the magnetic field, the induced current density, and the Lorentz force, which are usually followed in Eulerian frame, to those of the local Lyapunov exponents, which are naturally defined in Lagrangian coordinates.

  8. Banana regime pressure anisotropy in a bumpy cylinder magnetic field

    SciTech Connect

    Garcia-Perciante, A.L.; Callen, J.D.; Shaing, K.C.; Hegna, C.C.

    2006-01-15

    The pressure anisotropy is calculated for a plasma in a bumpy cylindrical magnetic field in the low collisionality (banana) regime for small magnetic-field modulations ({epsilon}{identical_to}{delta}B/2B<<1). Solutions are obtained by integrating the drift-kinetic equation along field lines in steady state. A closure for the local value of the parallel viscous force B{center_dot}{nabla}{center_dot}{pi}{sub parallel} is then calculated and is shown to exceed the flux-surface-averaged parallel viscous force by a factor of O(1/{epsilon}). A high-frequency limit ({omega}>>{nu}) for the pressure anisotropy is also determined and the calculation is then extended to include the full frequency dependence by using an expansion in Cordey eigenfunctions.

  9. Magnetic Anisotropy and Crystalline Electric Field in Quaternary Intermetallic Compounds

    NASA Astrophysics Data System (ADS)

    Lee, W. C.

    All isostructural compounds RNi2B2C (R =Er, Ho, Dy) show some magnetic transitions in magnetization isotherms at certain applied magnetic fields and temperatures above and below Neel and superconducting temperatures (TN, TC) where TN/TC varies from 0.57 to 1.66 for ErNi2B2C and DyNi2B2C. By using theoretical group analysis of D4h (I4/mmm) to the energy level scheme of crystalline electric field of magnetization isotherms anisotropy at various temperatures, we have obtained some possible ground state energy levels such as singlet Γ4 and first excited doublet state Γ5 in addition to another excited singlet Γ1 . Our crystalline electric field energy scheme analysis shows some qualitative agreement between theoretical calculation and experiments at high magnetic fields regime only, which means the interplay between antiferromagnetsm and superconductivity should be included. Magnetic Anisotropy and Crystalline Electric Field in Quaternary Intermetallic Compounds.

  10. Solar Surface Anisotropy effect on the Magnetic Field

    NASA Astrophysics Data System (ADS)

    Bommier, Véronique

    2015-10-01

    Within the literature there are at least 15 references indicating that the horizontal magnetic flux does not exactly balance vertical flux in sunspots, leading to the surprising result that div B would depart from zero. Intuitively, this has to be related to the stratification at the surface of the star, due to which horizontal and vertical typical lengths are different. This surface anisotropy results from gravity, but how does gravity influence the magnetic field? To answer this question, a scenario has been proposed in two recent publications, based on anisotropic Debye shielding. The presentation reported in this paper was devoted to investigate the possibility and causes of a non-zero div B. A scaling law associated with the anisotropy is able to reestablish the nullity of div B, which would lead to a renewed MHD in the solar photosphere layer. An eventual observation in the laboratory is also reported.

  11. Variance Anisotropy of Solar Wind Velocity and Magnetic Field Fluctuations

    NASA Astrophysics Data System (ADS)

    Oughton, S.; Matthaeus, W. H.; Wan, M.

    2015-12-01

    At MHD scales in the solar wind, velocity and magnetic fieldfluctuations are typically observed to have much more energy in thecomponents transverse to the mean magnetic field, relative to theparallel components [eg, 1,2]. This is often referred to asvariance anisotropy. Various explanations for it have been suggested,including that the fluctuations are predominantly shear Alfvén waves[1] and that turbulent dynamics leads to such states [eg, 3].Here we investigate the origin and strength of such varianceanisotropies, using spectral method simulations of thecompressible (polytropic) 3D MHD equations. We report on results from runs with several different classes ofinitial conditions. These classes include(i) fluctuations polarized only in the same sense as shear Alfvénwaves (aka toroidal polarization),(ii) randomly polarized fluctuations, and(iii) fluctuations restricted so that most of the energy is inmodes which have their wavevectors perpendicular, or nearly so, to thebackground magnetic field: quasi-2D modes. The plasma beta and Mach number dependence [4] of quantities like the variance anisotropy, Alfven ratio, and fraction of the energy in the toroidal fluctuations will be examined, along with the timescales for the development of any systematic features.Implications for solar wind fluctuations will be discussed. References:[1] Belcher & Davis 1971, J. Geophys. Res, 76, 3534.[2] Oughton et al 2015, Phil Trans Roy Soc A, 373, 20140152.[3] Matthaeus et al 1996, J. Geophys. Res, 101, 7619.[4] Smith et al 2006, J. Geophys. Res, 111, A09111.

  12. The manipulation of magnetic coercive field and orientation of magnetic anisotropy via electric fields

    NASA Astrophysics Data System (ADS)

    Xiang, Jun-Sen; Ye, Jun; Yang, Yun-Long; Xie, Yong; Li, Wei; Chen, Zi-Yu

    2016-08-01

    We report the effects of the electric field on the magnetic coercive field (H c) and uniaxial magnetic anisotropy (UMA) orientation of polycrystalline Ni film grown on an unpoled (0 1 1) [Pb(Mg1/3Nb2/3)O3](1‑x)–[PbTiO3] x (PMN-PT) single crystal substrate. Under various electric fields, normalized magnetic hysteresis loops of Ni films change in width; this represents the change of coercive field (ΔH c). Loop shapes are found to depend on the angle between the magnetic field and the sample, where changes in the shape reveal a small rotation of UMA. All these changes show that the magnetic properties vary periodically with a periodic electric field, by strain-mediated magnetoelectric coupling in the Ni/Ag/PMN-PT/Ag heterostructure. The poled PMN-PT produces strains under electric fields in the range of  ‑4.2 kV cm‑1  ⩽  E  ⩽  4.2 kV cm‑1, then transfers it to Ni films resulting in changes to its H c and UMA. The curves of the in-plane H c and strain, at two mutually orthogonal directions, represent butterfly patterns versus the applied electric field. In addition, the changes observed in both the H c and strain show asymmetric features in two orthogonal directions, which results in a small rotation angle of the UMA of Ni as the electric field decreases. The effective manipulation of magnitude and orientation of magnetic anisotropy via electric fields in ferromagnetic/ferroelectric (FM/FE) heterostructures is an important step towards controlling the magnetic tunnel junctions.

  13. Two-dimensional field-sensing map and magnetic anisotropy dispersion in magnetic tunnel junction arrays

    NASA Astrophysics Data System (ADS)

    Zhang, Wenzhe; Xiao, Gang; Carter, Matthew J.

    2011-04-01

    Due to the inherent disorder in local structures, anisotropy dispersion exists in almost all systems that consist of multiple magnetic tunnel junctions (MTJs). Aided by micromagnetic simulations based on the Stoner-Wohlfarth (S-W) model, we used a two-dimensional field-sensing map to study the effect of anisotropy dispersion in MTJ arrays. First, we recorded the field sensitivity value of an MTJ array as a function of the easy- and hard-axis bias fields, and then extracted the anisotropy dispersion in the array by comparing the experimental sensitivity map to the simulated map. Through a mean-square-error-based image processing technique, we found the best match for our experimental data, and assigned a pair of dispersion numbers (anisotropy angle and anisotropy constant) to the array. By varying each of the parameters one at a time, we were able to discover the dependence of field sensitivity on magnetoresistance ratio, coercivity, and magnetic anisotropy dispersion. The effects from possible edge domains are also discussed to account for a correction term in our analysis of anisotropy angle distribution using the S-W model. We believe this model is a useful tool for monitoring the formation and evolution of anisotropy dispersion in MTJ systems, and can facilitate better design of MTJ-based devices.

  14. Magnetic susceptibilities of V3+ in corundum: Magnetic anisotropy at high fields

    NASA Astrophysics Data System (ADS)

    Brumage, William H.; Quade, C. Richard; Dorman, C. Franklin

    1995-08-01

    We theoretically investigate the behavior of the V3+ ion as an impurity in Al2O3 under high magnetic fields, up to 20 T. In particular, we investigate the introduction of magnetic anisotropy that is lower than the trigonal symmetry of the host crystal. Two approaches are used for the calculations. First, fourth-order perturbation theory is used to develop quartic terms plus one sextic term in the susceptibility tensor that are good for fields up to 4 T. Then, the three-level energy matrix is reduced exactly to obtain the anisotropy at higher fields. It is found that the dominant contributions to the magnetic-induced anisotropy arise from the χxxxx term, while the χxxzz=χzxxz, χzzzz, and the χxxxxxx terms give a much lower contribution. Temperature-dependent effects are reported. There is a very small dependence of the magnetization upon the zero-field splitting.

  15. Field orientation dependence of magnetization reversal in thin films with perpendicular magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Fallarino, Lorenzo; Hovorka, Ondrej; Berger, Andreas

    2016-08-01

    The magnetization reversal process of hexagonal-close-packed (hcp) (0001) oriented Co and C o90R u10 thin films with perpendicular magnetic anisotropy (PMA) has been studied as a function of temperature and applied magnetic field angle. Room temperature pure cobalt exhibits two characteristic reversal mechanisms. For angles near in-plane field orientation, the magnetization reversal proceeds via instability of the uniform magnetic state, whereas in the vicinity of the out-of-plane (OP) orientation, magnetization inversion takes place by means of domain nucleation. Temperature dependent measurements enable the modification of the magnetocrystalline anisotropy and reveal a gradual disappearance of the domain nucleation process during magnetization reversal for elevated temperatures. Ultimately, this suppression of the domain nucleation process leads to the exclusive occurrence of uniform state instability reversal for all field orientations at sufficiently high temperature. Comparative magnetic measurements of C o90R u10 alloy samples allow the identification and confirmation of the high temperature remanent magnetization state of cobalt as an OP stripe domain state despite the reduction of magnetocrystalline anisotropy. Detailed micromagnetic simulations supplement the experimental results and corroborate the physical understanding of the temperature dependent behavior. Moreover, they enable a comprehensive identification of the complex energy balance in magnetic films with PMA, for which three different magnetic phases occur for sufficiently high anisotropy values, whose coexistence point is tricritical in nature.

  16. Exchange anisotropy determined by magnetic field dependence of ac susceptibility

    NASA Astrophysics Data System (ADS)

    Rodríguez-Suárez, R. L.; Vilela Leão, L. H.; de Aguiar, F. M.; Rezende, S. M.; Azevedo, A.

    2003-10-01

    ac susceptibility measurements of ferromagnetic/antiferromagnetic (FM/AF) bilayers are usually performed as a function of the temperature. In this work we describe measurements of transverse biased ac susceptibility (χt) of FM/AF bilayers as a function of the applied magnetic field H0. The measurements were carried out at room temperature by means of an ac magneto-optical Kerr effect susceptometer. The χt-1(H0) dependence, at the saturation magnetization regime, exhibits a linear behavior with the applied field parallel and perpendicular to the exchange bias direction. The linear extrapolation of χt-1 versus H0 cuts the abscissa at asymmetrical values of field due to the exchange bias coupling. The inverse susceptibility is calculated in the saturation regime by a model, which takes into account the free energy of both layers plus a term corresponding to the interfacial coupling. The exchange coupling field (HE) and uniaxial anisotropy (HU) are extracted from the best fit to the experimental results. The results obtained are crosschecked by those obtained from ferromagnetic resonance (FMR) and dc magnetometry. The measurements of the exchange bias and the uniaxial field in all of the three analyzed bilayers gave values that are consistently lower when measured by FMR than those obtained by ac and dc magnetometry. It is argued that the apparently discrepant values of HE and HU, obtained by different techniques, might be explained by existence of unstable AF grains at the AF/FM interface.

  17. A Way of Tailoring Magnetic Anisotropy of Co Nanowire Arrays: Magnetic Field Annealing.

    PubMed

    Ren, Yong; Qu, Li; Fan, Jiangxia; Dai, Bo; Wang, Jianbo

    2015-06-01

    Hexagonal close-packed Co nanowire arrays in anodic aluminum oxide template with the diameter of 50 nm have been fabricated using an ac electrodeposition method. The effect of magnetic field annealing on the thermal stability and magnetic properties of these nanwire arrays was studied. XRD measurements indicate the increase of diffraction intensity with the increase of heat-treatment temperature without magnetic field. Furthermore, the intensity of diffraction peak decreases rapidly if the sample undergoes the magnetic field annealing. Influence of different annealing process on the magnetic properties of Co nanowire arrays has also been studied. It is found that the magnetocrystalline anisotropy of hcp Co becomes weaker after magnetic field annealing, which lead to increase of the total anisotropy of Co nanowire arrays. PMID:26369071

  18. Manipulation of magnetic state in nanostructures by perpendicular anisotropy and magnetic field

    SciTech Connect

    Chen, J. P.; Xie, Y. L.; Chu, P.; Wang, Y. L.; Wang, Z. Q.; Gao, X. S.; Liu, J.-M.

    2014-06-28

    We investigate the transitions of spin configurations in ultrathin nanostructures by tuning the perpendicular anisotropy (K{sub z}) and out-of-plane magnetic field (H), using the Monte Carlo simulation. It is revealed that enhancing the anisotropy K{sub z} can drive the evolution of in-plane vortex state into intriguing saturated magnetization states under various H, such as the bubble domain state and quadruple-block-domain state etc. The spin configurations of these states exhibit remarkable H-dependence. In addition, the strong effects of geometry and size on the spin configurations of nanostructures are observed. In particular, a series of edged states occur in the circular disk-shaped lattices, and rich intricate saturated magnetization patterns appear in big lattices. It is suggested that the magnetic states can be manipulated by varying the perpendicular anisotropy, magnetic field, and geometry/size of the nanostructures. Furthermore, the stability (retention capacity) of the saturated magnetization states upon varying magnetic field is predicted, suggesting the potential applications of these saturated magnetization states in magnetic field-controlled data storages.

  19. Alignment of Iron Nanoparticles in a Magnetic Field Due to Shape Anisotropy

    DOE PAGESBeta

    Radhakrishnan, Balasubramaniam; Nicholson, Don M; Eisenbach, Markus; Ludtka, Gerard Michael; Rios, Orlando; Parish, Chad M

    2015-07-09

    During high magnetic field processing there is evidence for alignment of non-spherical metallic particles above the Curie temperature in alloys with negligible magneto-crystalline anisotropy. The main driving force for alignment is the magnetic shape anisotropy. Current understanding of the phenomenon is not adequate to quantify the effect of particle size, aspect ratio, temperature and the magnetic field on particle alignment. We demonstrate a Monte Carlo approach coupled with size scaling to show the conditions under which alignment is possible.

  20. Method and means for measuring the anisotropy of a plasma in a magnetic field

    DOEpatents

    Shohet, J.L.; Greene, D.G.S.

    1973-10-23

    Anisotropy is measured of a free-free-bremsstrahlungradiation-generating plasma in a magnetic field by collimating the free-free bremsstrahlung radiation in a direction normal to the magnetic field and scattering the collimated free- free bremsstrahlung radiation to resolve the radiation into its vector components in a plane parallel to the electric field of the bremsstrahlung radiation. The scattered vector components are counted at particular energy levels in a direction parallel to the magnetic field and also normal to the magnetic field of the plasma to provide a measure of anisotropy of the plasma. (Official Gazette)

  1. Inner Core Anisotropy Due to the Magnetic Field--induced Preferred Orientation of Iron.

    PubMed

    Karato, S

    1993-12-10

    Anisotropy of the inner core of the Earth is proposed to result from the lattice preferred orientation of anisotropic iron crystals during their solidification in the presence of a magnetic field. The resultant seismic anisotropy is related to the geometry of the magnetic field in the core. This hypothesis implies that the observed anisotropy (fast velocity along the rotation axis) indicates a strong toroidal field in the core, which supports a strong field model for the geodynamo if the inner core is made of hexagonal close-packed iron. PMID:17781788

  2. Magnetic field-dependent shape anisotropy in small patterned films studied using rotating magnetoresistance

    PubMed Central

    Fan, Xiaolong; Zhou, Hengan; Rao, Jinwei; Zhao, Xiaobing; Zhao, Jing; Zhang, Fengzhen; Xue, Desheng

    2015-01-01

    Based on the electric rotating magnetoresistance method, the shape anisotropy of a Co microstrip has been systematically investigated. We find that the shape anisotropy is dependent not only on the shape itself, but also on the magnetization distribution controlled by an applied magnetic field. Together with micro-magnetic simulations, we present a visualized picture of how non-uniform magnetization affects the values and polarities of the anisotropy constants and . From the perspective of potential appliantions, our results are useful in designing and understanding the performance of micro- and nano-scale patterned ferromagnetic units and the related device properties. PMID:26563520

  3. Current induced perpendicular-magnetic-anisotropy racetrack memory with magnetic field assistance

    SciTech Connect

    Zhang, Y.; Klein, J.-O.; Chappert, C.; Ravelosona, D.; Zhao, W. S.

    2014-01-20

    High current density is indispensable to shift domain walls (DWs) in magnetic nanowires, which limits the using of racetrack memory (RM) for low power and high density purposes. In this paper, we present perpendicular-magnetic-anisotropy (PMA) Co/Ni RM with global magnetic field assistance, which lowers the current density for DW motion. By using a compact model of PMA RM and 40 nm design kit, we perform mixed simulation to validate the functionality of this structure and analyze its density potential. Stochastic DW motion behavior has been taken into account and statistical Monte-Carlo simulations are carried out to evaluate its reliability performance.

  4. Field Variation of Low-field Anisotropy of Magnetic Susceptibility of Rocks: Measurement Problems

    NASA Astrophysics Data System (ADS)

    Hrouda, F.

    Theory of low-field anisotropy of magnetic susceptibility (AMS) assumes linear rela- tionship between magnetization and magnetizing field. This assumption is precisely valid in diamagnetic and paramagnetic minerals by definition, while in ferrimagnetic and antiferromagnetic minerals this relationship is in general non-linear, represented by hysteresis loop, being linear only in very weak fields in which the initial suscep- tibility is measured. Recently, it has been shown that, in using common measuring fields, the initial susceptibility is always measured in magnetite, while in pyrrhotite, hematite, and titanomagnetite the measured susceptibility may often be outside the initial susceptibility range. The field variation of low-field AMS results in lowering the quality of the fit of the susceptibility ellipsoid to the measured data and in mis- estimating the degree of anisotropy. Fortunately, the orientations of the principal sus- ceptibilities are virtually field-independent. The problem can be solved in basically three ways. The simplest way is using very weak measuring fields (less than 10 A/m), but this can result in significant lowering sensitivity and precision. The other way is to respect the non-linearity and measure the susceptibility in so many directions that contour diagram of directional susceptibilities can be presented instead of suscepti- bility ellipsoid. The third way is to measure the AMS in at least two fields within the Rayleigh law range and calculate the initial directional susceptibilities from which the AMS can be correctly determined using linear theory.

  5. Field-dependent perpendicular magnetic anisotropy in CoFeB thin films

    SciTech Connect

    Barsukov, I. Krivorotov, I. N.; Fu, Yu; Gonçalves, A. M.; Sampaio, L. C.; Spasova, M.; Farle, M.; Arias, R. E.

    2014-10-13

    We report ferromagnetic resonance measurements of perpendicular magnetic anisotropy in thin films of Ta/Co{sub 20}Fe{sub 60}B{sub 20}/MgO as a function of the Co{sub 20}Fe{sub 60}B{sub 20} layer thickness. The first and second order anisotropy terms show unexpectedly strong dependence on the external magnetic field applied to the system during the measurements. We propose strong interfacial spin pinning as a possible origin of the field-dependent anisotropy. Our results imply that high-field anisotropy measurements cannot be directly used for quantitative evaluation of zero-field performance parameters of CoFeB-based devices such as spin torque memory.

  6. Effects of anisotropies in turbulent magnetic diffusion in mean-field solar dynamo models

    SciTech Connect

    Pipin, V. V.; Kosovichev, A. G.

    2014-04-10

    We study how anisotropies of turbulent diffusion affect the evolution of large-scale magnetic fields and the dynamo process on the Sun. The effect of anisotropy is calculated in a mean-field magnetohydrodynamics framework assuming that triple correlations provide relaxation to the turbulent electromotive force (so-called the 'minimal τ-approximation'). We examine two types of mean-field dynamo models: the well-known benchmark flux-transport model and a distributed-dynamo model with a subsurface rotational shear layer. For both models, we investigate effects of the double- and triple-cell meridional circulation, recently suggested by helioseismology and numerical simulations. To characterize the anisotropy effects, we introduce a parameter of anisotropy as a ratio of the radial and horizontal intensities of turbulent mixing. It is found that the anisotropy affects the distribution of magnetic fields inside the convection zone. The concentration of the magnetic flux near the bottom and top boundaries of the convection zone is greater when the anisotropy is stronger. It is shown that the critical dynamo number and the dynamo period approach to constant values for large values of the anisotropy parameter. The anisotropy reduces the overlap of toroidal magnetic fields generated in subsequent dynamo cycles, in the time-latitude 'butterfly' diagram. If we assume that sunspots are formed in the vicinity of the subsurface shear layer, then the distributed dynamo model with the anisotropic diffusivity satisfies the observational constraints from helioseismology and is consistent with the value of effective turbulent diffusion estimated from the dynamics of surface magnetic fields.

  7. Leveraging intrinsic chain anisotropy to align coil-coil block copolymers with magnetic fields

    NASA Astrophysics Data System (ADS)

    Rokhlenko, Yekaterina; Zhang, Kai; Gopinadhan, Manesh; Larson, Steve; Majewski, Pawel; Yager, Kevin; Gopalan, Padma; O'Hern, Corey; Osuji, Chinedum

    Magnetic field alignment of block copolymers (BCPs) has typically relied on the presence of liquid crystalline or crystalline assemblies to provide sufficient magnetic anisotropy to drive alignment. Recent experiments however show that alignment is also possible in simple coil-coil BCPs. In particular, alignment of lamellae was observed in poly(styrene-b-4-vinylpyridine) (PS-P4VP) on cooling across the order-disorder transition at field strengths as low as 1 T, with alignment improving markedly with increasing field strength and decreasing cooling rate. Here we discuss the intrinsic chain anisotropy which drives the observed alignment, and its display as a net microdomain anisotropy due to chain tethering at the block interface. We use in-situ X-ray scattering to study the phase behavior and temperature-, time-, and field- dependent dynamics of magnetic alignment in coil-coil BCPs, highlighting the important roles of chain anisotropy and grain size in alignment. For the right combination of field strength and grain size, we can leverage intrinsic chain anisotropy to magnetically direct self-assembly in other coil-coil systems, including cylinder-forming poly(styrene-b-dimethylsiloxane). Field alignment of PS-P4VP with PEO and other blends provides a route to form functional materials such as nanoporous films and ion conducting polymers.

  8. Measuring remanence anisotropy of hematite in red beds: anisotropy of high-field isothermal remanence magnetization (hf-AIR)

    NASA Astrophysics Data System (ADS)

    Bilardello, Dario; Kodama, Kenneth P.

    2009-09-01

    The potential of using high-field anisotropy of isothermal remanence magnetization (hf-AIR) measurements for determining the origin of natural remanent magnetization in red beds and for identifying and correcting possible red-bed inclination shallowing was investigated for specimens of the Carboniferous Shepody Formation of New Brunswick and Nova Scotia, Canada. The technique makes it possible for a typical paleomagnetic laboratory to measure the remanence anisotropy of high-coercivity hematite. High-field (hf) AIR was used in conjunction with 100 mT alternating field (af) and 120°C thermal demagnetization to separate the contribution of hematite to the remanence anisotropy from that of magnetite/maghemite and goethite, respectively. A 5-T impulse DC magnetic field was used for the hf-AIR to reset the magnetic moment of high-coercivity hematite so that demagnetization between AIR orientations was not necessary. The ability of a 5-T field to reset the magnetization was tested by generating an isothermal remanent magnetization acquisition curve for hematite by using impulse DC magnetic fields up to 5 T in one orientation and followed by applying a field in the opposite direction at each step. Each field application was treated by 120°C heating and 100 mT af demagnetization before measurement. At 5 T, the difference between the magnetizations applied in opposite directions disappeared indicating that no magnetic memory persisted at this field strength. We performed a validity and reproducibility test of our hf-AIR measurement technique by measuring three specimens multiple times along two orthogonal coordinate systems. The method yielded highly reproducible results and, on rotating the specimen's coordinates, the fabric rotated by 90° as expected, showing that it is not an artifact of the technique. We also measured hf-AIR on samples that had previously been chemically demagnetized in 3N HCl to remove the secondary, chemically grown pigmentary hematite. The hf

  9. Investigations of cosmic ray anisotropies and their relationship to concurrent magnetic field data

    NASA Technical Reports Server (NTRS)

    Allum, F. R.

    1974-01-01

    Investigations of cosmic ray anisotropies and their relationship to concurrent magnetic field data are reported. These investigations range in scope from the examination of data very late in the decay phase of a solar particle event where long term (approximately 6 hour) averages are used and definite interplanetary effects sought after to an examination of the change in low energy particle anisotropy as the satellite approaches the bow shock and the magnetopause.

  10. Electric field controlled reversible magnetic anisotropy switching studied by spin rectification

    SciTech Connect

    Zhou, Hengan; Fan, Xiaolong Wang, Fenglong; Jiang, Changjun; Rao, Jinwei; Zhao, Xiaobing; Xue, Desheng; Gui, Y. S.; Hu, C.-M.

    2014-03-10

    In this letter, spin rectification was used to study the electric field controlled dynamic magnetic properties of the multiferroic composite which is a Co stripe with induced in-plane anisotropy deposited onto a Pb(Mg{sub 1∕3}Nb{sub 2∕3})O{sub 3}-PbTiO{sub 3} substrate. Due to the coupling between piezoelectric and magnetoelastic effects, a reversible in-plane anisotropy switching has been realized by varying the history of the applied electric field. This merit results from the electric hysteresis of the polarization in the nonlinear piezoelectric regime, which has been proved by a butterfly type electric field dependence of the in-plane anisotropy field. Moreover, the electric field dependent effective demagnetization field and linewidth have been observed at the same time.

  11. Determination of the electric field induced anisotropy change in sub-100 nm perpendicularly magnetized devices

    NASA Astrophysics Data System (ADS)

    Huang, Jiancheng; Tran, Michael; Lim, Sze Ter; Huang, Aihong; Yang, Chuyi; Yap, Qi Jia; Han, Guchang

    2016-05-01

    We measure the voltage or electric field (EF) modulated change in anisotropy using two methods on the same nanometer sized device: 1) Directly using the area of the hard axis magnetization loop and 2) Indirectly using the switching field distribution method. Both methods yield similar values of efficiency. With the indirect method, the efficiency derived from the thermal stability was found to be more consistent than that from the anisotropy field. Our data also suggests that memory devices that rely solely on EF effects may benefit from larger device sizes.

  12. ANISOTROPY AS A PROBE OF THE GALACTIC COSMIC-RAY PROPAGATION AND HALO MAGNETIC FIELD

    SciTech Connect

    Qu, Xiao-bo; Zhang, Yi; Liu, Cheng; Hu, Hong-bo; Xue, Liang

    2012-05-01

    The anisotropy of cosmic rays (CRs) in the solar vicinity is generally attributed to CR streaming due to the discrete distribution of CR sources or local magnetic field modulation. Recently, the two-dimensional large-scale CR anisotropy has been measured by many experiments in the TeV-PeV energy range in both hemispheres. The tail-in excess along the tangential direction of the local spiral arm and the loss cone deficit pointing to the north Galactic pole direction agree with what have been obtained in tens to hundreds of GeV. The persistence of the two large-scale anisotropy structures in such a wide energy range suggests that the anisotropy might be due to global streaming of the Galactic CRs (GCRs). This work tries to extend the observed CR anisotropy picture from the solar system to the whole galaxy. In such a case, we can find a new interesting signature, a loop of GCR streaming, of the GCR propagation. We further calculate the overall GCR streaming induced magnetic field, and find a qualitative consistency with the observed structure of the halo magnetic field.

  13. Tuning of the nucleation field in nanowires with perpendicular magnetic anisotropy

    SciTech Connect

    Kimling, Judith; Gerhardt, Theo; Kobs, Andre; Vogel, Andreas; Peter Oepen, Hans; Merkt, Ulrich; Meier, Guido; Wintz, Sebastian; Im, Mi-Young; Fischer, Peter

    2013-04-28

    We report on domain nucleation in nanowires consisting of Co/Pt multilayers with perpendicular magnetic anisotropy that are patterned by electron-beam lithography, sputter deposition, and lift-off processing. It is found that the nucleation field can be tuned by changing the geometry of the wire ends. A reduction of the nucleation field by up to 60% is achieved when the wire ends are designed as tips. This contrasts with the behavior of wires with in-plane anisotropy where the nucleation field increases when triangular-pointed ends are used. In order to clarify the origin of the reduction of the nucleation field, micromagnetic simulations are employed. The effect cannot be explained by the lateral geometrical variation but is attributable to a local reduction of the perpendicular anisotropy caused by shadowing effects due to the resist mask during sputter deposition of the multilayer.

  14. On the alignment of plasma anisotropies and the magnetic field direction in the solar wind

    NASA Technical Reports Server (NTRS)

    Asbridge, J. R.; Bame, S. J.; Feldman, W. C.; Gosling, J. T.; Ness, N. F.

    1977-01-01

    One year's Imp 6 solar wind plasma and magnetic field data are examined to determine whether anisotropies in particle velocity distributions are aligned with the measured interplanetary magnetic field vector. Alignment of components in the analysis plane was generally found to be excellent whenever plasma parameter magnitudes were larger than determination uncertainties, although some spread exists (typical rms approximately equal to 10 deg). By assuming cylindrical symmetry about the simultaneously measured magnetic field vector during the 1-year interval under study, three-dimensional values of selected solar wind plasma thermal parameters were constructed from the two-dimensional plasma measurements, and the statistical properties of their distributions have been tabulated.

  15. In-plane magnetic anisotropy and coercive field dependence upon thickness of CoFeB

    NASA Astrophysics Data System (ADS)

    Kipgen, Lalminthang; Fulara, Himanshu; Raju, M.; Chaudhary, Sujeet

    2012-09-01

    The structural and magnetic properties of as-grown 5-50 nm thin ion-beam sputter deposited transition metal-metalloid Co20Fe60B20 (CFB) films are reported in this communication. A broad peak observed at 2θ∼45° in the glancing angle X-ray diffraction pattern revealed the formation of very fine nano-sized grains embedded in majority amorphous CFB matrix. Although no magnetic field is applied during deposition, the longitudinal magneto-optic Kerr effect measurements performed at 300 K in these as-grown films clearly established the presence of in-plane uniaxial magnetic anisotropy (Ku). It is argued that this observed anisotropy is strain-induced. This is supported by the observed dependence of direction of Ku on the angle between applied magnetic field and crystallographic orientation of the underlying Si(100) substrate, and increase in the coercivity with the increase of the film thickness.

  16. MAGNETIC FIELDS AND COSMIC-RAY ANISOTROPIES AT TeV ENERGIES

    SciTech Connect

    Battaner, Eduardo; Castellano, Joaquín; Masip, Manuel E-mail: jcastellano@correo.ugr.es

    2015-02-01

    Several cosmic-ray (CR) observatories have provided high-accuracy maps of the sky at TeV-PeV energies. The data reveal an O(0.1%) deficit from north galactic directions that peaks at 10 TeV and then evolves with the energy, together with other anisotropies at smaller angular scales. Using the Boltzmann equation, we derive expressions for the CR flux that fit these features. The anisotropies depend on the local interstellar magnetic field B{sub IS}, on the average galactic field B{sub R} in our vicinity, and on correlations between fluctuating quantities. We show that the initial dipole anisotropy along B{sub IS} can be modulated by changes in the global CR flow, and that a variation in the dipole direction would imply a given radius of coherence for the local B{sub IS}. We also show that small- and medium-scale anisotropies may appear when the full-sky anisotropy finds a field configuration acting as a magnetic lens.

  17. Alignment of iron nanoparticles in a magnetic field due to shape anisotropy

    NASA Astrophysics Data System (ADS)

    Radhakrishnan, B.; Nicholson, D. M.; Eisenbach, M.; Parish, C.; Ludtka, G. M.; Rios, O.

    2015-11-01

    During high magnetic field solidification processing there is evidence for the alignment of nanoscale metallic particles with elongated morphologies that nucleate from a liquid metal. Such alignment occurs well above the Curie temperature of the particle where the magneto-crystalline anisotropy energy and exchange energy contributions are negligible. The main driving force for alignment is the magnetic shape anisotropy. Current understanding of the phenomenon is not adequate to quantify the effect of particle size, aspect ratio, temperature and the magnetic field on particle alignment. We demonstrate a Monte Carlo approach coupled with a scaling law for the dipole-dipole interaction energy as a function of the particle size to identify the conditions under which such alignment is possible.

  18. Effects of the galactic magnetic field upon large scale anisotropies of extragalactic cosmic rays

    SciTech Connect

    Harari, D.; Mollerach, S.; Roulet, E. E-mail: mollerach@cab.cnea.gov.ar

    2010-11-01

    The large scale pattern in the arrival directions of extragalactic cosmic rays that reach the Earth is different from that of the flux arriving to the halo of the Galaxy as a result of the propagation through the galactic magnetic field. Two different effects are relevant in this process: deflections of trajectories and (de)acceleration by the electric field component due to the galactic rotation. The deflection of the cosmic ray trajectories makes the flux intensity arriving to the halo from some direction to appear reaching the Earth from another direction. This applies to any intrinsic anisotropy in the extragalactic distribution or, even in the absence of intrinsic anisotropies, to the dipolar Compton-Getting anisotropy induced when the observer is moving with respect to the cosmic rays rest frame. For an observer moving with the solar system, cosmic rays traveling through far away regions of the Galaxy also experience an electric force coming from the relative motion (due to the rotation of the Galaxy) of the local system in which the field can be considered as being purely magnetic. This produces small changes in the particles momentum that can originate large scale anisotropies even for an isotropic extragalactic flux.

  19. Modification of the classical Heisenberg helimagnet by weak uniaxial anisotropy and magnetic field

    SciTech Connect

    Zaliznyak, I.A.; Zhitomirsky, M.E.

    1995-09-01

    A classical ground state of the isotropic Heisenberg spin Hamiltonian on a primitive Bravais lattice is known to be a single-Q plane helix. Additional uniaxial anisotropy and external magnetic field can greatly distort this structure by generating higher-order (at the wave vectors nQ) Fourier harmonics in the spatial spin configuration. These features are not captured within the usual formalism based on the Luttinger-Tisza theorem, when the classical ground state energy is minimized under the {open_quotes}weak{close_quotes} condition on the lengths of the spins. We discuss why the correct solution is lost in that approach and present another microscopic treatment of the problem. For easy-axis and easy-plane quadratic uniaxial anisotropy it allows one to find the classical ground state for general Q and for any orientation of the magnetic field considering the effect of anisotropy (but not the field) as a perturbation of the exchange structure. As a result, the classical ground state energy, the uniform magnetization, and the magnetic Bragg peak intensities that are measured in the experiments are calculated. 21 refs., 1 fig.

  20. Speed of field-driven domain walls in nanowires with large transverse magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Depassier, M. C.

    2015-07-01

    Recent analytical and numerical work on field-driven domain wall propagation in nanowires and thin films has shown that for large transverse anisotropy and sufficiently large applied fields the Walker profile becomes unstable before the breakdown field, giving way to a domain wall whose speed increases at a slower rate with the applied field. We perform an asymptotic expansion of the Landau-Lifshitz-Gilbert equation for large transverse magnetic anisotropy and show that the asymptotic dynamics reproduces this behavior. The appearance of a different regime in the asymptotic dynamics is due to a transition from a pushed to a pulled front of a reaction diffusion equation in which the speed of the domain wall increases with the square root of the applied field

  1. Probing the Intergalactic Magnetic Field with the Anisotropy of the Extragalactic Gamma-Ray Background

    NASA Technical Reports Server (NTRS)

    Venters, T. M.; Pavlidou, V.

    2012-01-01

    The intergalactic magnetic field (IGMF) may leave an imprint on the anisotropy properties of the extragalactic gamma-ray background, through its effect on electromagnetic cascades triggered by interactions between very high energy photons and the extragalactic background light. A strong IGMF will deflect secondary particles produced in these cascades and will thus tend to isotropize lower energy cascade photons, thus inducing a modulation in the anisotropy energy spectrum of the gamma-ray background. Here we present a simple, proof-of-concept calculation of the magnitude of this effect and demonstrate that the two extreme cases (zero IGMF and IGMF strong enough to completely isotropize cascade photons) would be separable by ten years of Fermi observations and reasonable model parameters for the gamma-ray background. The anisotropy energy spectrum of the Fermi gamma-ray background could thus be used as a probe of the IGMF strength.

  2. Probing the Intergalactic Magnetic Field with the Anisotropy of the Extragalactic Gamma-ray Background

    NASA Technical Reports Server (NTRS)

    Venters, T. M.; Pavlidou, V.

    2013-01-01

    The intergalactic magnetic field (IGMF) may leave an imprint on the angular anisotropy of the extragalactic gamma-ray background through its effect on electromagnetic cascades triggered by interactions between very high energy photons and the extragalactic background light. A strong IGMF will deflect secondary particles produced in these cascades and will thus tend to isotropize lower energy cascade photons, thereby inducing a modulation in the anisotropy energy spectrum of the gamma-ray background. Here we present a simple, proof-of-concept calculation of the magnitude of this effect and demonstrate that current Fermi data already seem to prefer nonnegligible IGMF values. The anisotropy energy spectrum of the Fermi gamma-ray background could thus be used as a probe of the IGMF strength.

  3. Hale cycle effects in cosmic ray east-west anisotropy and interplanetary magnetic field

    NASA Technical Reports Server (NTRS)

    Ahluwalia, H. S.

    1993-01-01

    We have reanalyzed diurnal anisotropy data obtained with the shielded ion chamber (IC) at Cheltenham/Fredericksburg and the neutron monitor (NM) at Swarthmore/Newark. IC data are for the 1936-1977 period and NM data are for the 1965-1988 period. We have corrected IC data for the diurnal temperature effect. Application of this correction results in a better agreement between IC and other data sets, thereby making it possible to study the long-term changes in the diurnal anisotropy using IC data. The behavior of the annual mean east-west anisotropy is studied for 53 years of observations. The period encompasses more than two solar magnetic (Hale) cycles. Its amplitude undergoes the expected 11 and 22 year variations, with the largest changes occurring near solar activity minima. Moreover, the data indicate the presence of the subsidiary maxima for the entire 53-year period, following the solar polar field reversals, during the declining phases of activity cycles when high-speed solar wind streams are present in the heliosphere. The data suggest that the amplitude of the subsidiary maximum is large when the solar polar magnetic field points toward the sun in the Northern Hemisphere, and radial anisotropy is absent.

  4. Anisotropy of the Vortex Magnetic Field Distribution in LuNi2B2

    NASA Astrophysics Data System (ADS)

    Eskildsen, M. R.; Debeer-Schmitt, L.; Rovira, K.; Jenkins, N.; Dewhurst, C. D.; Bud'Ko, S. L.; Canfield, P. C.

    2008-03-01

    It is well known that the vortex lattice (VL) symmetry and orientation in type-II superconductors is very sensitive to any anisotropy within the screening current plane. A classic example is the sequence of transitions from hexagonal to rhombic to square symmetry, which was first observed in the borocarbide superconductors and explained by a Fermi surface anisotropy coupled with the non-local electrodynamics responsible for vortex-vortex interactions. Recently, however, this is mounting experimental evidence for a strong gap anisotropy and possible point nodes in the basal plane of these materials. Here we report on small-angle neutron scattering studies of the VL in a carefully annealed, high quality LuNi2B2C single crystal, which permitted us to measure the VL form factor for a large number of reflections. These measurements allow a reconstruction of the real space profile of the magnetic field around the vortices, reflecting the basal plane anisotropy of the screening currents in LuNi2B2C. The results will be compared to predictions for both Fermi surface and gap anisotropies, and will serve as a valuable reference for more complicated compounds as e.g. Sr2RuO4, heavy fermions and high-Tc's.

  5. Effect of MgO/Fe Interface Oxidation State on Electric-Field Modulation of Interfacial Magnetic Anisotropy

    NASA Astrophysics Data System (ADS)

    Guan, X. W.; Cheng, X. M.; Wang, S.; Huang, T.; Xue, K. H.; Miao, X. S.

    2016-06-01

    The impact of the MgO/Fe interface oxidation state on the electric-field-modified magnetic anisotropy in MgO/Fe has been revealed by density functional calculations. It is shown that the influence of the interface oxidation is strong enough to dominate the effect of the electric field on the magnetic anisotropy of MgO/Fe-based films. The magnetoelectric coefficients are calculated to be positive for the ideal and overoxidized MgO/Fe interface, but an abnormal negative value emerges in the underoxidized case. By analyzing the interface states based on density of states and band structures, we demonstrate that the considerably different electronic structures of the three oxidized MgO/Fe interfaces lead to the strong discrepancy in the electric-field modulation of the interfacial magnetic anisotropy. These results are of considerable interest in the area of electric-field-controlled magnetic anisotropy and switching.

  6. Effect of MgO/Fe Interface Oxidation State on Electric-Field Modulation of Interfacial Magnetic Anisotropy

    NASA Astrophysics Data System (ADS)

    Guan, X. W.; Cheng, X. M.; Wang, S.; Huang, T.; Xue, K. H.; Miao, X. S.

    2016-03-01

    The impact of the MgO/Fe interface oxidation state on the electric-field-modified magnetic anisotropy in MgO/Fe has been revealed by density functional calculations. It is shown that the influence of the interface oxidation is strong enough to dominate the effect of the electric field on the magnetic anisotropy of MgO/Fe-based films. The magnetoelectric coefficients are calculated to be positive for the ideal and overoxidized MgO/Fe interface, but an abnormal negative value emerges in the underoxidized case. By analyzing the interface states based on density of states and band structures, we demonstrate that the considerably different electronic structures of the three oxidized MgO/Fe interfaces lead to the strong discrepancy in the electric-field modulation of the interfacial magnetic anisotropy. These results are of considerable interest in the area of electric-field-controlled magnetic anisotropy and switching.

  7. Magnetic multilayer interface anisotropy

    SciTech Connect

    Pechan, M.J.

    1992-01-01

    Ni/Mo and Ni/V multilayer magnetic anisotropy has been investigated as a function of Ni layer thickness, frequency and temperature. Variable frequency ferromagnetic resonance (FMR) measurements show, for the first time, significant frequency dependence associated with the multilayer magnetic anisotropy. The thickness dependence allows one to extract the interface contribution from the total anisotropy. Temperature dependent FMR (9 GHz) and room temperature magnetization indicate that strain between Ni and the non-magnetic layers is contributing significantly to the source of the interface anisotropy and the state of the interfacial magnetization. In order to examine the interface properties of other transition metal multilayer systems, investigations on Fe/Cu are underway and CoCr/Ag is being proposed. ESR measurements have been reported on Gd substituted YBaCuO superconductors and a novel quasi-equilibrium method has been developed to determine quickly and precisely the ransition temperature.

  8. Pressure-anisotropy-driven microturbulence and magnetic-field evolution in shearing, collisionless plasma

    NASA Astrophysics Data System (ADS)

    Melville, Scott; Schekochihin, Alexander A.; Kunz, Matthew W.

    2016-07-01

    The non-linear state of a high-beta collisionless plasma is investigated where an imposed shear amplifies or diminishes a uniform mean magnetic field, driving pressure anisotropies and, therefore, firehose or mirror instabilities. To mimic the local behaviour of a macroscopic flow, the shear is switched off or reversed after one shear time, so a new macroscale configuration is superimposed on previous microscale state. A threshold plasma beta is found: when β ≪ Ω/S (ion cyclotron frequency/shear rate), the emergence/disappearance of firehose or mirror fluctuations is quasi-instantaneous compared to the shear time (lending some credence to popular closures that assume this). This follows from the free decay of these fluctuations being constrained by the same marginal-stability conditions as their growth in the unstable regime, giving the decay time ˜β/Ω ≪ S-1. In contrast, when β ≳ Ω/S, the old microscale state only disappears on the shear time-scale. In this `ultra-high-beta' regime, driven firehose fluctuations grow secularly to order-unity amplitudes, compensating for the decrease of the mean field and thus pinning the pressure anisotropy at marginal stability without scattering particles - unlike what happens at moderate β. After the shear reverses, the shearing away of these fluctuations compensates for the increase of the mean field and thus prevents growth of the pressure anisotropy, so the system stays close to the firehose threshold, does not go mirror-unstable, the total magnetic energy barely changing at all. Implications for various astrophysical situations, especially the origin of cosmic magnetism, are discussed: collisionless effects appear mostly beneficial to fast magnetic-field generation.

  9. Anisotropy in Magnetism

    NASA Astrophysics Data System (ADS)

    Baberschke, Klaus

    The enormous research on magnetic properties of ultrathin films and nanostructures produces also new activities in the fundamental understanding of the magnetic anisotropy energy (MAE) and the anisotropy of the orbital magnetic momentapprox 0.05\\ Å. This small change in structure and symmetry increa ses the MAE by several orders of magnitude and lifts the quenching of the orbital moment. Increases of 20-30 % of the orbital moment mu _{L} are observed. This experimental finding is confirmed by full relativistic ab initio calculations. Various experiments deliver the full temperature dependence of all MAE contributions. The temperature dependence remains a challenge for the theory in itine rant magnetism.

  10. Anatomy of electric field control of perpendicular magnetic anisotropy at Fe/MgO interfaces

    NASA Astrophysics Data System (ADS)

    Ibrahim, F.; Yang, H. X.; Hallal, A.; Dieny, B.; Chshiev, M.

    2016-01-01

    The charge-mediated effect of electric field on the perpendicular magnetic anisotropy (PMA) of Fe/MgO interfaces is investigated using first-principles calculations. We present an approach by discussing this effect in relation to the intrinsic dipole field existing at the Fe/MgO interface. A firm correlation between the PMA and the interfacial dipole is established and further verified in the absence of an applied electric field. The on-site projected PMA analysis not only elucidates that the effect of electric field on the PMA extends beyond the interfacial Fe layer, but also shows that the second Fe layer carries the largest contribution to the effect. This observation is interpreted in relation to the orbital hybridization changes induced by applying an electric field.

  11. Combined effect of demagnetizing field and induced magnetic anisotropy on the magnetic properties of manganese-zinc ferrite composites

    NASA Astrophysics Data System (ADS)

    Babayan, V.; Kazantseva, N. E.; Moučka, R.; Sapurina, I.; Spivak, Yu. M.; Moshnikov, V. A.

    2012-01-01

    This work is devoted to the analysis of factors responsible for the high-frequency shift of the complex permeability (μ*) dispersion region in polymer composites of manganese-zinc (MnZn) ferrite, as well as to the increase in their thermomagnetic stability. The magnetic spectra of the ferrite and its composites with polyurethane (MnZn-PU) and polyaniline (MnZn-PANI) are measured in the frequency range from 1 MHz to 3 GHz in a longitudinal magnetization field of up to 700 Ое and in the temperature interval from -20 °С to +150 °С. The approximation of the magnetic spectra by a model, which takes into account the role of domain wall motion and magnetization rotation, allows one to determine the specific contribution of resonance processes associated with domain wall motion and the natural ferromagnetic resonance to the μ*. It is established that, at high frequencies, the μ* of the MnZn ferrite is determined solely by magnetization rotation, which occurs in the region of natural ferromagnetic resonance when the ferrite is in the “single domain” state. In the polymer composites of the MnZn ferrite, the high-frequency permeability is also determined mainly by the magnetization rotation; however, up to high values of magnetizing fields, there is a contribution of domain wall motion, thus the “single domain” state in ferrite is not reached. The frequency and temperature dependence of μ* in polymer composites are governed by demagnetizing field and the induced magnetic anisotropy. The contribution of the induced magnetic anisotropy is crucial for MnZn-PANI. It is attributed to the elastic stresses that arise due to the domain wall pinning by a polyaniline film adsorbed on the surface of the ferrite during in-situ polymerization.

  12. Attempts to Simulate Anisotropies of Solar Wind Fluctuations Using MHD with a Turning Magnetic Field

    NASA Technical Reports Server (NTRS)

    Ghosh, Sanjoy; Roberts, D. Aaron

    2010-01-01

    We examine a "two-component" model of the solar wind to see if any of the observed anisotropies of the fields can be explained in light of the need for various quantities, such as the magnetic minimum variance direction, to turn along with the Parker spiral. Previous results used a 3-D MHD spectral code to show that neither Q2D nor slab-wave components will turn their wave vectors in a turning Parker-like field, and that nonlinear interactions between the components are required to reproduce observations. In these new simulations we use higher resolution in both decaying and driven cases, and with and without a turning background field, to see what, if any, conditions lead to variance anisotropies similar to observations. We focus especially on the middle spectral range, and not the energy-containing scales, of the simulation for comparison with the solar wind. Preliminary results have shown that it is very difficult to produce the required variances with a turbulent cascade.

  13. Petrophysical Characterization of Stony Meteorites Using Low Field Magnetic Susceptibility: Initial Results From Anisotropy Measurements

    NASA Astrophysics Data System (ADS)

    Smith, D. L.; Ernst, R. E.; Herd, R. K.; Claire, S.

    2004-05-01

    Low field magnetic susceptibility represents a fast, systematic and non-destructive technique of meteorite classification [1-4]. We previously reported measurements of bulk susceptibility, and its frequency dependence, along with a `proxy' measure of anisotropy, on 204 specimens from 108 different meteorites in the National Meteorite Collection of Canada [5,6]. Measurements were performed on a Sapphire Instruments Model 2B. Bulk susceptibility values followed expected trends, governed by metal content, with values increasing from LL, to L, to H, to E chondrites. Frequency dependence (19000 vs 825 Hz) was greatest in H and C chondrites. Aubrites (AUB) and Howardites (HOW) had the lowest. Anisotropy of magnetic susceptibility (AMS) was measured using a `proxy' approach: the mean value determined from a series of random sample orientations was compared with repeated measurements in one orientation. AUB, E chondrites and Martian SNCs had the largest inferred anisotropies, while LL and C chondrites had the lowest. Here we report initial results from a follow-up study. Quantitative measurements of the AMS were made on 67 stony meteorite specimens. AMS measurements [3,5,6,7,8,9] can provide information on the physical fabric of the meteorite, and may relate to its deformational history. Samples measured show significant degrees of anisotropy ranging from 1-50 % for an individual specimen (in parentheses is the number of specimens used in the class mean): AUB (5), Acapulcoites (1) and E chondrites (10) display the largest degrees of anisotropy, 40±11 (1 standard deviation), 34, and 24±10, respectively. These classes are followed by Diogenite (1) 20, H (13) 14±7 and L (10) 13±6 chondrites, Brachinite (1) 11, Ureilite (2) 8, Eucrite (4) 7±4, C chondrites (14) 6±3, and Rumurutiite (1) 4. These results match a similar trend based on the `proxy' method [5,6]: AUB and E chondrites were found to have the highest inferred anisotropies followed by tightly grouped H and L

  14. Orientational dynamics of ferrofluids with finite magnetic anisotropy of the particles: relaxation of magneto-birefringence in crossed fields.

    PubMed

    Raikher, Yu L; Stepanov, V I; Bacri, J-C; Perzynski, R

    2002-08-01

    Dynamic birefringence in a ferrofluid subjected to crossed bias (constant) and probing (pulse or ac) fields is considered, assuming that the nanoparticles have finite magnetic anisotropy. This is done on the basis of the general Fokker-Planck equation that takes into account both internal magnetic and external mechanical degrees of freedom of the particle. We describe the orientation dynamics in terms of the integral relaxation time of the macroscopic orientation order parameter. To account for an arbitrary relation between the bias (external) and anisotropy (internal) fields, an interpolation expression for the integral relaxation time is proposed and justified. A developed description is used to interpret the measurements of birefringence relaxation in magnetic fluids with nanoparticles of high (cobalt ferrite) and low (maghemite) anisotropy. The proposed theory appears to be in full qualitative agreement with all the experimental data available. PMID:12241160

  15. Anisotropy of 2G HTS racetrack coils in external magnetic fields

    NASA Astrophysics Data System (ADS)

    Chudy, Michal; Chen, Yiran; Zhang, Min; Coombs, T. A.

    2013-07-01

    Pancake or racetrack coils wound with second generation high-temperature superconductors (2G HTSs) are important elements for numerous applications of HTS. The applications of these coils are primarily in rotating machines such as motors and generators where they must withstand external magnetic fields from various orientations. The characterization of 2G HTS coils is mostly focused on AC loss assessment, critical current and maximum magnetic field evaluation. In this study, racetrack coils will be placed in different orientations of external magnetic fields—Jc (Ic) versus angle measurements will be performed and interpreted. Full attention is paid to studies of anisotropy Jc versus angle curves for short samples of 2G HTS tapes. As will be shown, the shape of the Jc versus angle curves for tapes has a strong influence on the Jc (Ic) versus angle curves for coils. In this work, a unique and unpredicted behavior of the Jc versus angle curves for the 2G HTS racetrack coils was found. This will be analyzed and fully explained.

  16. Effect of residual strain in Fe-based amorphous alloys on field induced magnetic anisotropy and domain structure

    NASA Astrophysics Data System (ADS)

    Azuma, Daichi; Hasegawa, Ryusuke; Saito, Shin; Takahashi, Migaku

    2013-05-01

    Field induced magnetic anisotropy in two Fe-based amorphous alloys with different saturation induction levels (1.56 T and 1.64 T) was investigated by varying magnetic field strength and annealing temperature and domain images were taken on these samples. Residual strain was evaluated by measuring coercivities of the materials after stress-relief annealing. These results are discussed, clarifying the difference between the two Fe-based amorphous alloys.

  17. Ru/FeCoB double layered film with high in-plane magnetic anisotropy field of 500 Oe

    NASA Astrophysics Data System (ADS)

    Hirata, Ken-ichiro; Hashimoto, Atsuto; Matsuu, Toshimitsu; Nakagawa, Shigeki

    2009-04-01

    FeCoB layers prepared on Ru underlayer possess a high saturation magnetization Ms and a high in-plane magnetic anisotropy filed Hk. Effects of preparation conditions were investigated. Low Ar gas pressure condition and thicker film thickness were effective to attain distortion of FeCo crystallite. As the crystallinity of Ru underlayer became higher, higher Hk was induced. The accumulation of anisotropic stress in the film caused by the oblique incidences of depositing atoms with high energy seems to be one of the important effects to attain high anisotropy field. It was succeeded to prepare the Ru/FeCoB film with high Hk of 500 Oe.

  18. Measurement of magnetostriction and induced magnetic anisotropy by SAMR method in Co-rich stress + field annealed amorphous ribbons

    NASA Astrophysics Data System (ADS)

    Blanco, J. M.; González, J.; Vázquez, M.; Barandiarán, J. M.; Hernando, A.

    1991-10-01

    The saturation magnetostriction (λ s) and induced magnetic anisotropy ( Kind) in (Co 0.95Fe 0.05) 80Si 10B 10 annealed amorphous alloy ribbons have been measured at room temperature with the SAMR (small-angle magnetization rotation) method. The ribbons were annealed under simulataneous action of a stress and/or magnetic field. The variations of λ s and Kind show parallel trends in the cases of stress and stress+field annealings but not for single field annealing. These variations are connected with microstructural changes originated during the treatments.

  19. Magnetic anisotropy and crystalline electric field effects in RRh{sub 4}B{sub 4} single crystals.

    SciTech Connect

    Zhou, H.; Lambert, S. E.; Maple, M. B.; Dunlap, B. D.; Materials Science Division; Univ. of California at San Diego

    2009-08-01

    Research on polycrystalline RRh{sub 4}B{sub 4} samples has shown that crystalline electric field (CEF) effects play an important role in these compounds. The successful synthesis of single crystal samples of RRh{sub 4}B{sub 4} with R = Y, Sm, Gd, Tb, Dy, Ho, Er, Tm, and Lu has provided an opportunity to further investigate CEF effects in these materials. Magnetization and magnetic susceptibility measurements on the RRh{sub 4}B{sub 4} single crystals revealed strong magnetic anisotropy, and the experimental results could be described well by CEF calculations based on the parameters derived from an analysis of experimental data for ErRh{sub 4}B{sub 4} single crystals. The easy directions of magnetization of these compounds are consistent with the signs of the Stevens factor {alpha}J of the CEF Hamiltonian. A strong influence of magnetic anisotropy on superconductivity was also observed.

  20. Intrinsic surface magnetic anisotropy in Y3Fe5O12 as the origin of low-magnetic-field behavior of the spin Seebeck effect

    NASA Astrophysics Data System (ADS)

    Uchida, Ken-ichi; Ohe, Jun-ichiro; Kikkawa, Takashi; Daimon, Shunsuke; Hou, Dazhi; Qiu, Zhiyong; Saitoh, Eiji

    2015-07-01

    The magnetic-field dependence of the longitudinal spin Seebeck effect (LSSE) in a Pt /Y3Fe5O12 (YIG)-slab junction system was found to deviate from a bulk magnetization curve of the YIG slab in a low field range. In this paper, we show that the deviation originates from the difference between surface and bulk magnetization processes in the YIG slab and that it appears even when removing possible extrinsic magnetic anisotropy due to surface roughness and replacing the Pt layer with different materials. This result indicates that the anomalous field dependence of the LSSE is due to an intrinsic magnetic property of the YIG surface. Our numerical calculation based on the Landau-Lifshitz-Gilbert equation shows that the deviation between the LSSE and bulk magnetization curves is qualitatively explained by introducing easy-axis perpendicular magnetic anisotropy near the surface of YIG.

  1. Electric field control of the magnetic anisotropy energy of double-vacancy graphene decorated by iridium atoms.

    PubMed

    Ge, Gui-Xian; Li, Ying-Bin; Wang, Guang-Hou; Wan, Jian-Guo

    2016-04-20

    To solve the fundamental dilemma in data storage applications, it is crucial to manipulate the magnetic anisotropy energy (MAE). Herein, using first-principles calculations, we predict that the system of double-vacancy graphene decorated by iridium atoms possesses high stability, giant MAE, perpendicular-anisotropy and long-range ferromagnetic coupling. More importantly, the amplitude of MAE can be manipulated by electric fields. This is due to the change in the occupation number of Ir-5d orbitals. The present hybrid system could be a high-performance nanoscale information storage device with ultralow energy consumption. PMID:27063394

  2. Broken symmetry approach to density functional calculation of magnetic anisotropy or zero field splittings for multinuclear complexes with antiferromagnetic coupling.

    PubMed

    van Wüllen, Christoph

    2009-10-29

    Antiferromagnetic coupling in multinuclear transition metal complexes usually leads to electronic ground states that cannot be described by a single Slater determinant and that are therefore difficult to describe by Kohn-Sham density functional methods. Density functional calculations in such cases are usually converged to broken symmetry solutions which break spin and, in many cases, also spatial symmetry. While a procedure exists to extract isotropic Heisenberg (exchange) coupling constants from such calculations, no such approach is yet established for the calculation of magnetic anisotropy energies or zero field splitting parameters. This work proposes such a procedure. The broken symmetry solutions are not only used to extract the exchange couplings but also single-ion D tensors which are then used to construct a (phenomenological) spin Hamiltonian, from which the magnetic anisotropy and the zero-field energy levels can be computed. The procedure is demonstrated for a bi- and a trinuclear Mn(III) model compound. PMID:19708660

  3. Direct measurement of the magnetic anisotropy field in Mn-Ga and Mn-Co-Ga Heusler films

    NASA Astrophysics Data System (ADS)

    Fowley, Ciarán; Ouardi, Siham; Kubota, Takahide; Yildirim, Oguz; Neudert, Andreas; Lenz, Kilian; Sluka, Volker; Lindner, Jürgen; Law, Joseph M.; Mizukami, Shigemi; Fecher, Gerhard H.; Felser, Claudia; Deac, Alina M.

    2015-04-01

    The static and dynamic magnetic properties of tetragonally distorted Mn-Ga based alloys were investigated. Static properties are determined in magnetic fields up to 6.5 T using SQUID magnetometry. For the pure Mn1.6Ga film, the saturation magnetisation is 0.36 MA m-1 and the coercivity is 0.29 T. Partial substitution of Mn by Co results in Mn2.6Co0.3Ga1.1. The saturation magnetisation of those films drops to 0.2 MA m-1 and the coercivity is increased to 1 T. The time-resolved magneto-optical Kerr effect (TR-MOKE) is used to probe the high-frequency dynamics of Mn-Ga. The ferromagnetic resonance frequency extrapolated to zero-field is found to be 125 GHz with a Gilbert damping, α, of 0.019. The anisotropy field is determined from both SQUID and TR-MOKE to be 4.5 T, corresponding to an effective anisotropy density of 0.81 MJ m-3. Given the large anisotropy field of the Mn2.6Co0.3Ga1.1 film, pulsed magnetic fields up to 60 T are used to determine the field strength required to saturate the film in the plane. For this, the extraordinary Hall effect was employed as a probe of the local magnetisation. By integrating the reconstructed in-plane magnetisation curve, the effective anisotropy energy density for Mn2.6Co0.3Ga1.1 is determined to be 1.23 MJ m-3.

  4. Periodic magnetic domain wall pinning in an ultrathin film with perpendicular anisotropy generated by the stray magnetic field of a ferromagnetic nanodot array

    NASA Astrophysics Data System (ADS)

    Metaxas, P. J.; Zermatten, P.-J.; Jamet, J.-P.; Ferré, J.; Gaudin, G.; Rodmacq, B.; Schuhl, A.; Stamps, R. L.

    2009-03-01

    The stray magnetic field of an array of hard ferromagnetic perpendicularly magnetized [Co/Pt]4 nanodots is used to nondestructively generate a periodic pinning potential for domain walls in an underlying [Pt/Co]2/Pt layer with perpendicular anisotropy. Pinning is evidenced using magneto-optical microscopy. The magnetic field (H) dependence of the average wall velocity in the presence of the periodic pinning potential is consistent with thermally activated creep, modified only by the addition of a uniform retarding field Hret, whose magnitude depends on the relative alignment of H and the dots' magnetizations.

  5. Irreversible magnetic processes under biaxial and uniaxial magnetic anisotropies

    NASA Astrophysics Data System (ADS)

    Pokharel, S.; Akioya, O.; Alqhtany, N. H.; Dickens, C.; Morgan, W.; Wuttig, M.; Lisfi, A.

    2016-05-01

    Irreversible magnetic processes have been investigated in magnetic systems with two different anisotropy symmetries (uniaxial and biaxial) through angular measurement of the switching field, the irreversible susceptibility and the magnetic viscosity. These two systems consist of two-dimensional cobalt ferrite hetero-structures epitaxially grown on (100) and (110) MgO substrate. It is found that for uniaxial anisotropy the irreversible characteristics of the magnetization are large and display a strong angular dependence, which exhibits its maximum at the easy axis and drops quickly to vanish at the hard axis. However, for biaxial anisotropy the magnetization irreversible characteristics are considerably reduced and are less sensitive to the field angle.

  6. Ru/FeCoB double layered film with high in-plane magnetic anisotropy field of 500 Oe

    SciTech Connect

    Hirata, Ken-ichiro; Hashimoto, Atsuto; Matsuu, Toshimitsu; Nakagawa, Shigeki

    2009-04-01

    FeCoB layers prepared on Ru underlayer possess a high saturation magnetization M{sub s} and a high in-plane magnetic anisotropy filed H{sub k}. Effects of preparation conditions were investigated. Low Ar gas pressure condition and thicker film thickness were effective to attain distortion of FeCo crystallite. As the crystallinity of Ru underlayer became higher, higher H{sub k} was induced. The accumulation of anisotropic stress in the film caused by the oblique incidences of depositing atoms with high energy seems to be one of the important effects to attain high anisotropy field. It was succeeded to prepare the Ru/FeCoB film with high H{sub k} of 500 Oe.

  7. Intrinsic anisotropy-defined magnetization reversal in submicron ring magnets

    NASA Astrophysics Data System (ADS)

    Li, S. P.; Lew, W. S.; Bland, J. A. C.; Natali, M.; Lebib, A.; Chen, Y.

    2002-12-01

    We report a study of the effect of magnetocrystalline anisotropy in the magnetization reversal of submicron Co rings fabricated by nanoimprint lithography. For weak magnetocrystalline anisotropy, the complete reversal takes place via a transition from saturation at large negative fields, into a vortex configuration at small fields, and back to reverse saturation at large positive fields. When the anisotropy strength is increased to a critical value, the intermediate vortex configuration no longer exists in the magnetization reversal along the easy axis; instead, the reversal occurs through a rapid jump. However, when the applied field direction is far from the easy axis, the presence of the magnetocrystalline anisotropy favors local vortex nucleation, and this leads to a similar switching process as found for low anisotropy. Micromagnetic simulations indicate that the magnetization reversal process of the rings, starts from a buckling-like reverse domain nucleation, followed by local vortex formation and an avalanche process of local vortex nucleation.

  8. Electric field modulation of magnetic anisotropy and microwave absorption properties in Fe50Ni50/Teflon composite films

    NASA Astrophysics Data System (ADS)

    Xia, Zhenjun; He, Jun; Ou, Xiulong; Wang, Yu; He, Shuli; Zhao, Dongliang; Yu, Guanghua

    2016-05-01

    Fe50Ni50 nanoparticle films with the size about 6 nm were deposited by a high energetic cluster deposition source. An electric field of about 0 - 40 kV was applied on the sample platform when the films were prepared. The field assisted deposition technique can dramatically induce in-plane magnetic anisotropy. To probe the microwave absorption properties, the Fe50Ni50 nanoparticles were deliberately deposited on the dielectric Teflon sheet. Then the laminated Fe50Ni50/Teflon composites were used to do reflection loss scan. The results prove that the application of electric field is an effective avenue to improve the GHz microwave absorption performance of our magnetic nanoparticles films expressed by the movement of reflection loss peak to high GHz region for the composites.

  9. Small-scale primordial magnetic fields and anisotropies in the cosmic microwave background radiation

    SciTech Connect

    Jedamzik, Karsten; Abel, Tom E-mail: tabel@slac.stanford.edu

    2013-10-01

    It is shown that small-scale magnetic fields present before recombination induce baryonic density inhomogeneities of appreciable magnitude. The presence of such inhomogeneities changes the ionization history of the Universe, which in turn decreases the angular scale of the Doppler peaks and increases Silk damping by photon diffusion. This unique signature could be used to (dis)prove the existence of primordial magnetic fields of strength as small as B ≅ 10{sup −11} Gauss by cosmic microwave background observations.

  10. CMB temperature anisotropy at large scales induced by a causal primordial magnetic field

    SciTech Connect

    Bonvin, Camille; Caprini, Chiara E-mail: camille.bonvin@cea.fr

    2010-05-01

    We present an analytical derivation of the Sachs Wolfe effect sourced by a primordial magnetic field. In order to consistently specify the initial conditions, we assume that the magnetic field is generated by a causal process, namely a first order phase transition in the early universe. As for the topological defects case, we apply the general relativistic junction conditions to match the perturbation variables before and after the phase transition which generates the magnetic field, in such a way that the total energy momentum tensor is conserved across the transition and Einstein's equations are satisfied. We further solve the evolution equations for the metric and fluid perturbations at large scales analytically including neutrinos, and derive the magnetic Sachs Wolfe effect. We find that the relevant contribution to the magnetic Sachs Wolfe effect comes from the metric perturbations at next-to-leading order in the large scale limit. The leading order term is in fact strongly suppressed due to the presence of free-streaming neutrinos. We derive the neutrino compensation effect dynamically and confirm that the magnetic Sachs Wolfe spectrum from a causal magnetic field behaves as l(l+1) C{sup B}{sub l}∝l{sup 2} as found in the latest numerical analyses.

  11. A correlation of energetic particle flux anisotropies with magnetic field variations in- and outside the coma of Comet Halley

    NASA Astrophysics Data System (ADS)

    Kirsch, E.; McKenna-Lawlor, S.; Ip, W.-H.; Daly, P. W.; Thompson, A.; O'Sullivan, D.; Neubauer, F. M.

    Anisotropies and energy spectra of cometary ions derived from the EPA/EPONA measurements on board of Giotto during the encounter with Comet Halley are used to study the acceleration processes taking place in the vicinity of the comet. Further evidence was found for the second order Fermi process. The intensity spikes observed outside the bowshock (outbound) can most likely be explained by the field line merging process at the frontside of the magnetic pileup region. The shock drift acceleration mechanism combined with the first order Fermi process seems to be responsible for the spike observed at 06:45 - 08:00 UT on March 14, 1986. The observed flux anisotropies are caused by the velocity transformation effect. Furthermore it can be concluded that the magnetic field lines were 'open' on the inbound side (19:00 - 23:00 UT on March 13), whereas a field line connection between cometary and interplanetary field lines must have existed on the outbound side until about 07:00 UT on March 14, 1986.

  12. SWAP operation in the two-qubit Heisenberg XXZ model: Effects of anisotropy and magnetic field

    SciTech Connect

    Zhou Yue; Yang Fuhua; Feng Songlin; Zhang Guofeng

    2007-06-15

    In this paper we study the SWAP operation in a two-qubit anisotropic XXZ model in the presence of an inhomogeneous magnetic field. We establish the range of anisotropic parameter {lambda} within which the SWAP operation is feasible. The SWAP errors caused by the inhomogeneous field are evaluated.

  13. The Large Scale Structure of the Galactic Magnetic Field and High Energy Cosmic Ray Anisotropy

    NASA Astrophysics Data System (ADS)

    Alvarez-Muñiz, Jaime; Stanev, Todor

    2006-10-01

    Measurements of the magnetic field in our Galaxy are complex and usually difficult to interpret. A spiral regular field in the disk is favored by observations, however the number of field reversals is still under debate. Measurements of the parity of the field across the Galactic plane are also very difficult due to the presence of the disk field itself. In this work we demonstrate that cosmic ray protons in the energy range 1018 to 1019eV, if accelerated near the center of the Galaxy, are sensitive to the large scale structure of the Galactic Magnetic Field (GMF). In particular if the field is of even parity, and the spiral field is bi-symmetric (BSS), ultra high energy protons will predominantly come from the Southern Galactic hemisphere, and predominantly from the Northern Galactic hemisphere if the field is of even parity and axi-symmetric (ASS). There is no sensitivity to the BSS or ASS configurations if the field is of odd parity.

  14. Ru/FeCoB crystalline soft magnetic underlayers with high anisotropy field for CoPtCr-SiO2 granular perpendicular magnetic recording media

    NASA Astrophysics Data System (ADS)

    Matsuu, Toshimitsu; Hirata, Ken-ichiro; Hashimoto, Atsuto; Matsunuma, Satoshi; Inoue, Tetsutaro; Doi, Tsugihiro; Nakagawa, Shigeki

    2009-04-01

    Ru/FeCoB/Ru/CoPtCr-SiO2 films were fabricated as perpendicular magnetic recording media with crystalline soft magnetic underlayer (SUL). Ru/FeCoB layers possessed high in-plane anisotropy field Hk of 400 Oe and a bcc-FeCo (110) orientation. Crystalline orientation of the FeCoB in the SUL affected on a crystallite growth of a Ru intermediate layer deposited on it and on crystallite orientation of the CoPtCr-SiO2 film deposited on the Ru intermediate layer. Ru/CoPtCr-SiO2 films without Ru/FeCoB SULs exhibited a random orientation of Ru crystallites and the in-plane magnetic anisotropy. On the other hand, Ru/CoPtCr-SiO2 films deposited on the Ru/FeCoB SULs exhibited (001) preferential orientations of the CoPtCr as well as the Ru intermediate layer and possessed perpendicular magnetic anisotropy. It was confirmed that the improvement of a bcc-FeCo (110) orientation in the SUL was effective to the improvement of a hcp-Ru (001) orientation. At the media for an intermediate layer thickness of 5 nm, the similar magnetic properties as that of 30 nm were obtained. It indicated that the application of a crystalline SUL promoted the reduction in the intermediate layer thickness.

  15. Magnetocrystalline anisotropy and its electric-field-assisted switching of Heusler-compound-based perpendicular magnetic tunnel junctions

    NASA Astrophysics Data System (ADS)

    Bai, Zhaoqiang; Shen, Lei; Cai, Yongqing; Wu, Qingyun; Zeng, Minggang; Han, Guchang; Feng, Yuan Ping

    2014-10-01

    Employing density functional theory combined with the non-equilibrium Green's function formalism, we systematically investigate the structural, magnetic and magnetoelectric properties of the Co2FeAl(CFA)/MgO interface, as well as the spin-dependent transport characteristics of the CFA/MgO/CFA perpendicular magnetic tunnel junctions (p-MTJs). We find that the structure of the CFA/MgO interface with the oxygen-top FeAl termination has high thermal stability, which is protected by the thermodynamic equilibrium limit. Furthermore, this structure is found to have perpendicular magnetocrystalline anisotropy (MCA). Giant electric-field-assisted modifications of this interfacial MCA through magnetoelectric coupling are demonstrated with an MCA coefficient of up to 10-7 erg V-1 cm. In addition, our non-collinear spin transport calculations of the CFA/MgO/CFA p-MTJ predict a good magnetoresistance performance of the device.

  16. Recording performance and thermal stability in perpendicular media with enhancement of grain isolation as well as magnetic anisotropy field

    NASA Astrophysics Data System (ADS)

    Jung, H. S.; Ikeda, Y.; Choe, G.; Shi, Zhupei

    2012-04-01

    Magnetic clustering, thermal stability, and recording performance on perpendicular media with multilayered magnetic anisotropy field (Hk)-gradient CoPtCr-oxide/Cap layers with various Ru-oxide layer thicknesses (tRu-oxide) on top of Ru/NiW layers are investigated. With increasing tRu-oxide from 0 to 1.3 nm, Hc and Hs are enhanced but Hn is reduced. Magnetic correlation length (Dn) extracted from a set of major and minor loops significantly decreases but intrinsic switching field distribution remains unaffected. A short-time switching field (Ho) proportional to Hk increases linearly while KuV/kT remains unchanged. Similar KuV/kT is explained by compensation of the reduced Dn with the enhanced Ku induced by a thin Ru-oxide. However, thermal decay rate degrades from 0.06 to 0.32%/decade, which correlates well with Hn. Similar values of initial minor loop slopes indicate no change in magnetic switching behavior. A 1 nm-thick Ru-oxide layer as a well-defined granular template significantly improves recording performance: narrower MCW at 10 T by 8 nm and higher SNR at 2 T by 1.4 dB are observed even at lower OW by 8 dB compared to the media without Ru-oxide. All the recording parameters as a function of Dn correlate well.

  17. The effect of magnetization anisotropy and paramagnetic susceptibility on the magnetization process

    NASA Astrophysics Data System (ADS)

    Bolyachkin, A. S.; Neznakhin, D. S.; Bartashevich, M. I.

    2015-12-01

    The Sucksmith-Thompson method is a widespread technique for the accurate evaluation of magnetocrystalline anisotropy constants K1 and K2 of a single crystal with easy magnetization axis or basal plane type magnetic anisotropy. In this work, a generalized form of the method is represented. It takes into account several magnetization process features: spontaneous magnetization anisotropy, high-field differential susceptibility (paramagnetic process), and stray fields in terms of the demagnetizing factor. Corrected anisotropy field expressions for both magnetic anisotropy types are also established herein. The modified approach was verified by magnetization measurements of single crystalline LaCo5 and YFe3.

  18. Slow magnetic relaxation in octahedral cobalt(II) field-induced single-ion magnet with positive axial and large rhombic anisotropy.

    PubMed

    Herchel, Radovan; Váhovská, Lucia; Potočňák, Ivan; Trávníček, Zdeněk

    2014-06-16

    Pseudooctahedral mononuclear cobat(II) complex [Co(abpt)2(tcm)2] (1), where abpt = 4-amino-3,5-bis(2-pyridyl)-1,2,4-triazole and tcm = tricyanomethanide anion, shows field-induced slow relaxation of magnetization with U = 86.2 K and large axial and rhombic single-ion zero-field-splitting parameters, D = +48(2) cm(-1) and E/D = 0.27(2) (D = +53.7 cm(-1) and E/D = 0.29 from ab initio CASSCF/NEVPT2 calculations), thus presenting a new example of a field-induced single-ion magnet with transversal magnetic anisotropy. PMID:24853769

  19. Magnetic anisotropy of strained epitaxial manganite films

    SciTech Connect

    Demidov, V. V. Borisenko, I. V.; Klimov, A. A.; Ovsyannikov, G. A.; Petrzhik, A. M.; Nikitov, S. A.

    2011-05-15

    The in-plane magnetic anisotropy of epitaxial La{sub 0.7}Sr{sub 0.3}MnO{sub 3} (LSMO) films is studied at room temperature by the following three independent techniques: magnetooptical Kerr effect, ferromagnetic resonance at a frequency of 9.61 GHz, and recording of absorption spectra of electromagnetic radiation at a frequency of 290.6 MHz. The films are deposited onto NdGaO{sub 3} (NGO) substrates in which the (110)NGO plane is tilted at an angle of 0-25.7 Degree-Sign to the substrate plane. The uniaxial magnetic anisotropy induced by the strain of the film is found to increase with the tilt angle of the (110)NGO plane. A model is proposed to describe the change in the magnetic anisotropy energy with the tilt angle. A sharp increase in the radio-frequency absorption in a narrow angular range of a dc magnetic field near a hard magnetization axis is detected The anisotropy parameters of the LSMO films grown on (110)NGO, (001)SrTiO{sub 3}, and (001)[(LaAlO{sub 3}){sub 0.3} + (Sr{sub 2}AlTaO{sub 6}){sub 0.7}] substrates are compared.

  20. Cotton-mouton effects, magnetic hyperpolarizabilities, and magnetic anisotropies of the methyl halides. Comparison with molecular Zeeman and high-field NMR spectroscopic results

    SciTech Connect

    Coonan, M.H.; Ritchie, G.L.D. )

    1991-02-07

    Measurements of the vapor-phase Cotton-Mouton effects of methyl fluoride, methyl bromide, and methyl iodide are reported. Analysis of the results, in conjunction with those of an earlier study of methane and methyl chloride, shows that in the series CH{sub 3}X (X = H, F, Cl, Br, I) the magnetic hyperpolarizabiity anisotropy, which is related to the quadratic response of the molecular polarizability to a magnetic field, is positive in sign and roughly proportional in magnitude to the mean polarizability. The magnetic anisotropies (10{sup 29}{Delta}{sub {chi}}/J T{sup {minus}2}) found for methyl chloride,methyl bromide, and methyl iodide (CH{sub 3}Cl, {minus}15.0 {plus minus} 1.3; CH{sub 3}Br, -15.1 {plus minus} 0.8; CH{sub 3}I, {minus}18.0 {plus minus} 1.5) are compared with values obtained by the molecular Zeeman and high-field {sup 2}H NMR spectroscopic methods.

  1. Effects of external magnetic field and magnetic anisotropy on chiral spin structures of square nanodisks investigated with a quantum simulation approach

    NASA Astrophysics Data System (ADS)

    Liu, Zhaosen; Ian, Hou

    2016-04-01

    We employed a quantum simulation approach to investigate the magnetic properties of monolayer square nanodisks with Dzyaloshinsky-Moriya (DM) interaction. The computational program converged very quickly, and generated chiral spin structures on the disk planes with good symmetry. When the DM interaction is sufficiently strong, multi-domain structures appears, their sizes or average distance between each pair of domains can be approximately described by a modified grid theory. We further found that the external magnetic field and uniaxial magnetic anisotropy both normal to the disk plane lead to reductions of the total free energy and total energy of the nanosystems, thus are able to stabilize and/or induce the vortical structures, however, the chirality of the vortex is still determined by the sign of the DM interaction parameter. Moreover, the geometric shape of the nanodisk affects the spin configuration on the disk plane as well.

  2. Microstructural, Magnetic Anisotropy, and Magnetic Domain Structure Correlations in Epitaxial FePd Thin Films with Perpendicular Magnetic Anisotropy

    NASA Technical Reports Server (NTRS)

    Skuza, J. R.; Clavero, C.; Yang, K.; Wincheski, B.; Lukaszew, R. A.

    2009-01-01

    L1(sub 0)-ordered FePd epitaxial thin films were prepared using dc magnetron sputter deposition on MgO (001) substrates. The films were grown with varying thickness and degree of chemical order to investigate the interplay between the microstructure, magnetic anisotropy, and magnetic domain structure. The experimentally measured domain size/period and magnetic anisotropy in this high perpendicular anisotropy system were found to be correlated following the analytical energy model proposed by Kooy and Enz that considers a delicate balance between the domain wall energy and the demagnetizing stray field energy.

  3. Electric field control of anisotropy and magnetization switching in CoFe and CoNi thin films for magnetoelectric memory devices

    NASA Astrophysics Data System (ADS)

    Jin, Tianli; Hao, Liang; Cao, Jiangwei; Liu, Mingfeng; Dang, Honggang; Wang, Ying; Wu, Dongping; Bai, Jianmin; Wei, Fulin

    2014-04-01

    We report on the marked change in magnetic anisotropy and magnetization reversal in Co50Fe50/[Pb(Mg1/3Nb2/3O3)]1-x-[PbTiO3]x (PMN-PT) and Co43Ni57/PMN-PT heterostructures under an electric field. For the Co50Fe50/PMN-PT structure, the electric-field-induced magnetic anisotropy field can be as large as 1.2 kOe at 12 kV/cm, corresponding to a magnetoelectric coefficient of 100 Oe cm/kV. In the Co43Ni57/PMN-PT heterostructure, the electric-field-induced anisotropy has a sign opposite to that in Co50Fe50/PMN-PT. As a result, in the [CoNi/Cu/CoFe/Cu]n/PMN-PT heterostructure, the parallel magnetic moment between two magnetic layers in the initial state may become perpendicular under an electric field. On the basis of these discussions, a voltage-write magnetoelectric memory device model is proposed.

  4. Electric field control of magnetic anisotropy in the easy cone state of Ta/Pt/CoFeB/MgO structures

    NASA Astrophysics Data System (ADS)

    Park, Kyung-Woong; Park, June-Young; Baek, Seung-heon Chris; Kim, Dae-Hoon; Seo, Soo-Man; Chung, Sung-Woong; Park, Byong-Guk

    2016-07-01

    The electric-field control of magnetic anisotropy is of particular interest because it allows the manipulation of the magnetization direction in spintronic devices with high performance and low power consumption. In this work, we investigate the effect of an electric field on the magnetic anisotropy in Ta/Pt/CoFeB/MgO structures, whose easy axis of magnetization is canted from the z-axis, forming a cone state. When an electric field is applied to the sample, its anisotropy constants change, thus modulating the cone state. It is demonstrated that the cone angle is controlled between 22° and 32° by a bias field of 4 MV/cm and that it can persist even after removing the bias. Moreover, it fully recovers to the original value when a bias voltage with an opposite polarity is applied. The non-volatile and reversible control of the cone state paves the way towards the utilization of the magnetic cone state in spintronic devices.

  5. Magnetic anisotropy of ferrosmectic phases

    NASA Astrophysics Data System (ADS)

    Ponsinet, Virginie; Fabre, Pascale; Veyssié, Madeleine; Cabanel, Régis

    1994-10-01

    A new anisotropic magnetic fluid, called ferrosmectic, is obtained when using a colloidal suspension of submicronic magnetic particles (ferrofluid), as a component in a smectic phase of fluid membranes. These lamellar phases present specific magnetic properties. The anisotropy of their magnetic susceptilities as a function of particles concentration is studied and interpreted : a microscopic mechanism involving a steric hindrance between particles and membranes is used to understand the experimental results. Un nouveau fluide magnétique anisotrope, appelé ferrosmectique, est obtenu lorsque nous utilisons un ferrofluide, c'est-à-dire une suspension colloïdale de particules magnétiques de taille inférieure au micron, comme composant dans la fabrication d'une phase smectique de membranes fluides. Ces phases adoptent des comportements spécifiques sous champ magnétique, et nous présentons ici une étude de l'anisotropie de leur susceptibilité magnétique en fonction de la concentration en particules. Nous interprétons les résultats obtenus par un mécanisme microscopique basé sur l'existence d'une gêne stérique entre membranes et particules.

  6. Advanced magnetic anisotropy determination through isothermal remanent magnetization of nanoparticles

    NASA Astrophysics Data System (ADS)

    Hillion, A.; Tamion, A.; Tournus, F.; Gaier, O.; Bonet, E.; Albin, C.; Dupuis, V.

    2013-09-01

    We propose a theoretical framework enabling the simulation of isothermal remanence magnetization (IRM) curves, based on the Stoner-Wohlfarth model combined with the Néel macrospin relaxation time description. We show how low temperature IRM curves, which have many advantages compared to hysteresis loops, can be efficiently computed for realistic assemblies of magnetic particles with both a size and anisotropy constant distribution, and a biaxial anisotropy. The IRM curves, which probe the irreversible switching provoked by an applied field, are shown to be complementary to other usual measurements (in particular low-field susceptibility curves where a thermal switching is involved). As an application, the experimental IRM curve of Co clusters embedded in a carbon matrix is analyzed. We demonstrate how powerful such an analysis can be, which in the present case allows us to put into evidence an anisotropy constant dispersion among the Co nanoparticles.

  7. THE EFFECTS OF PLASMA BETA AND ANISOTROPY INSTABILITIES ON THE DYNAMICS OF RECONNECTING MAGNETIC FIELDS IN THE HELIOSHEATH

    SciTech Connect

    Schoeffler, K. M.; Drake, J. F.; Swisdak, M.

    2011-12-10

    The plasma {beta} (the ratio of the plasma pressure to the magnetic pressure) of a system can have a large effect on its dynamics as high {beta} enhances the effects of pressure anisotropies. We investigate the effects of {beta} in a system of stacked current sheets that break up into magnetic islands due to magnetic reconnection, which is analogous to the compressed heliospheric current sheet in the heliosheath. We find significant differences between systems with low and high initial values of {beta}. At low {beta}, growing magnetic islands are modestly elongated and become round as contraction releases magnetic stress and reduces magnetic energy. At high {beta}, the increase of the parallel pressure in contracting islands causes saturation of modestly elongated islands as island cores approach the marginal firehose condition. Only highly elongated islands reach finite size. The anisotropy within these islands prevents full contraction, leading to a final state of highly elongated islands in which further reconnection is suppressed. The elongation of islands at finite {beta} is further enhanced by reducing the electron-to-ion mass ratio to more realistic values. The results are directly relevant to reconnection in the sectored region of the heliosheath where there is evidence that elongated islands are present, and possibly to other high-{beta} systems such as astrophysical accretion flows and the magnetosphere of Saturn.

  8. Large electric-field control of perpendicular magnetic anisotropy in strained [Co/Ni] / PZT heterostructures

    NASA Astrophysics Data System (ADS)

    Gopman, Daniel; Dennis, Cindi; Chen, P. J.; Iunin, Yury; Shull, Robert

    We present a piezoelectric/ferromagnetic heterostructure with PMA - a Co/Ni multilayer sputtered directly onto a Pb(Zr,Ti)O3 (PZT) substrate. Chemical-mechanical polishing was used to reduce the roughness of PZT plates to below 2 nm rms, enabling optimal magnetoelectric coupling via the direct interface between PZT and sputtered Co/Ni films with large PMA (Keff = (95 +/-9 kJ/m3)) . We grew the following layer stack: Ta(3)/Pt(2)/[Co(0.15)/Ni(0.6)]x4/Co(0.15)/Pt(2)/Ta(3); numbers in parentheses indicate thicknesses in nm. Applied electric fields up to +/- 2 MV/m to the PZT generated 0.05% in-plane compression in the Co/Ni multilayer, enabling a large electric-field reduction of the PMA (ΔKeff >= 103 J/m3) and of the coercive field (35%). Our results demonstrate that: (i) heterostructures combining PZT and [Co/Ni] exhibit larger PMA (Keff ~105 J/m3) than previous magnetoelectric heterostructures based on Co/Pt and CoFeB, enabling thermally stable hybrid magnetoelectric/spintronic devices only tens of nm in diameter and (ii) electric-field control of the PMA is promising for more energy efficient switching of spintronic devices.

  9. Magnetic Domain Confinement by Anisotropy Modulation

    NASA Astrophysics Data System (ADS)

    Li, S. P.; Lew, W. S.; Bland, J. A.; Lopez-Diaz, L.; Vaz, C. A.; Natali, M.; Chen, Y.

    2002-02-01

    The spin configuration in a magnet is in general a ``natural'' consequence of both the intrinsic properties of the material and the sample dimensions. We demonstrate that this limitation can be overcome in a homogeneous ferromagnetic film by engineering an anisotropy contrast. Substrates with laterally modulated single-crystal and polycrystalline surface regions were used to induce selective epitaxial growth of a ferromagnetic Ni film. The resulting spatially varying magnetic anisotropy leads to regular perpendicular and in-plane magnetic domains, separated by a new type of magnetic wall-the ``anisotropy constrained'' magnetic wall.

  10. Growth anisotropy effect of bulk high temperature superconductors on the levitation performance in the applied magnetic field

    NASA Astrophysics Data System (ADS)

    Zheng, J.; Liao, X. L.; Jing, H. L.; Deng, Z. G.; Yen, F.; Wang, S. Y.; Wang, J. S.

    2013-10-01

    Growth anisotropies of bulk high temperature superconductors (HTSCs) fabricated by a top-seeded melt texture growth process, that is, different pinning effect in the growth sectors (GSs) and growth sector boundaries (GSBs), possess effect on the macro flux trapping and levitation performance of bulk HTSCs. Previous work (Physics Procedia, 36 (2012) 1043) has found that the bulk HTSC array with aligned GSB pattern (AGSBP) exhibits better capability for levitation and suppression of levitation force decay above a permanent magnet guideway (PMG) compared with misaligned GSB pattern (MGSBP). In this paper, we further examine this growth anisotropy effect on the maglev performance of a double-layer bulk HTSC. In contrast to reported trapped flux cases (Supercond. Sci. Technol. 19 (2006) S466), the two superposed bulk HTSCs with same AGSBP with PMG are found to show better maglev performance. These series of results are helpful and support a new way for the performance optimization of present HTS maglev systems.

  11. The influence of magnetic aftereffects on the magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Mashukov, A.; Mashukova, A.

    2012-04-01

    There were investigated the time dependences of the magnetic anisotropy characteristics of artificial depositions received in the geomagnetic field. The content of magnetite in the nonmagnetic matrix of kaolin did not exceed 1%. The Co content in the grains of magnetite Fe3 O4 was 0.0018%. The viscous magnetization was created in the depositions with grain sizes of Fe3O4 in micrometers (0 ÷ 8), (9 ÷ 16), (17 ÷ 32), (33 ÷ 64), (65 ÷ 100), (101 ÷ 150). The X-ray method of direct pole figures indicates that the intensity of the ordering of the ferromagnetic grains in the depositions depends strongly on the grain size in the above-mentioned ranges, getting reduced from 1.9 to 1.1. Compared with the characteristics received immediately after drying the samples and after holding them for two years in the earth's magnetic field in the direction of In, one could observe increase in all the characteristics of the magnetic anisotropy. The magnitude Hd of the magnetic field having the periodicity change of Hd 2π to π increases. This indicates the stabilization of the new domain structure. The increase in the uniaxial anisotropy constant (K) is associated with the emergence of the large induced anisotropy due to the diffusion of Co ions. It was found out that the constant K decreases markedly with increasing particle size in the range from 8 mm to 40 microns. Based on the results of the X-ray analysis by using the method direct pole figures, it may be explained by the creation of the axial texture in the depositions with grains having the size less than 40 microns. The intensity of more than 40 microns decreases insignificantly - from 1.3 to 1.1. After creating the viscous magnetization in two years, the constant K has increased by 1.5 - 2 times. The influence of the magnetic after-effects on K in strong magnetic fields denotes the diffusion nature of the viscous magnetization. The losses of the rotational magnetic hysteresis (W) also rise in the presence of the

  12. Magnetic properties and anisotropy in magnetic thin films and superlattices

    NASA Astrophysics Data System (ADS)

    Guo, Wenli

    A systematic study of the magnetic properties and anisotropy in magnetic thin films as well as superlattices is presented in this thesis. The main objective is to investigate by means of the Green function technique the order-disorder phase transition and reorientation transition in a non-perturbative microscopic theory valid in the whole temperature range of interest. We consider the magnetic systems that may consist of an arbitrary number of layers with any spin. We start with a discussion of general properties and origins of anisotropies of the magnetic systems, and a list of questions that we are trying to answer. A comparison between different theoretical approaches follows. The Green function method is used to derive analytical expressions for various anisotropies. The energy spectrum and the spontaneous magnetization are obtained as well. Based on these results, the transition temperature and the Curie temperature are calculated as functions of the Fe film thickness. It is shown that the condition for the reorientation transition is equivalent to that for the zero energy gap at the bottom of the spin-wave spectrum. Special features under the influence of normal external field, anisotropic exchange couplings and next-nearest-neighbor couplings on the magnetization reorientation of magnetic thin films are then investigated in detail. It is demonstrated that the nature of perpendicular remanent (PR) depends primarily on the surface anisotropy and film thickness. The magnetic properties of Tb/Fe superlattices are also studied. It shows ferrimagnetic properties and normal uniaxial anisotropy. An approximation is proposed to treat magnetic Ni films of arbitrary thickness and arbitrary lattice structure for general spin. It is a much simpler way of calculation, in which one does not have to solve the determinant equation, especially the one with off-diagonal elements. The temperature and thickness dependence of various anisotropies are then investigated. There

  13. Anisotropy of MHD Turbulence at Low Magnetic Reynolds Number

    NASA Technical Reports Server (NTRS)

    Zikanov, O.; Vorobev, A.; Thess, A.; Davidson, P. A.; Knaepen, B.

    2004-01-01

    Turbulent fluctuations in MHD flows are known to become dimensionally anisotropic under the action of a sufficiently strong magnetic field. We consider the technologically relevant case of low magnetic Reynolds number and apply the method of DNS of forced flow in a periodic box to generate velocity fields. The analysis based on different anisotropy characteristics shows that the dimensional anisotropy is virtually scale-independent. We also find that, except for the case of very strong magnetic field, the flow is componentally isotropic. Its kinetic energy is practically uniformly distributed among the velocity components.

  14. Temperature memory of the induced magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Vetcfinski, V. S.; Tunyi, I.

    2012-04-01

    Methods of higher harmonics applied to study the effects associated with the induced magnetic anisotropy (IMA) of ferro- and ferrimagnetic materials are considered. Physical processes causing the anisotropy and small value of these effects are analyzed. It is demonstrated that the IMA can remember the pressure at which it was formed.

  15. ANISOTROPY DETERMINATIONS IN EXCHANGE SPRING MAGNETS.

    SciTech Connect

    LEWIS,L.H.; HARLAND,C.L.

    2002-08-18

    Ferromagnetic nanocomposites, or ''exchange spring'' magnets, possess a nanoscaled microstructure that allows intergrain magnetic exchange forces to couple the constituent grains and alter the system's effective magnetic anisotropies. While the effects of the anisotropy alterations are clearly seen in macroscopic magnetic measurement, it is extremely difficult to determine the detailed effects of the system's exchange coupling, such as the interphase exchange length, the inherent domain wall widths or the effective anisotropies of the system. Clarification of these materials parameters may be obtained from the ''micromagnetic'' phenomenological model, where the assumption of magnetic reversal initiating in the magnetically-soft regions of the exchange-spring maqet is explicitly included. This approach differs from that typically applied by other researchers and allows a quantitative estimate of the effective anisotropies of an exchange spring system. Hysteresis loops measured on well-characterized nanocomposite alloys based on the composition Nd{sub 2}Fe{sub 14}B + {alpha}-Fe at temperatures above the spin reorientation temperature were analyzed within the framework of the micromagnetic phenomenological model. Preliminary results indicate that the effective anisotropy constant in the material is intermediate to that of bulk {alpha}-Fe and bulk Nd{sub 2}Fe{sub 14}B and increases with decreasing temperature. These results strongly support the idea that magnetic reversal in nanocomposite systems initiates in the lower-anisotropy regions of the system, and that the soft-phase regions become exchange-hardened by virtue of their proximity to the magnetically-hard regions.

  16. Slow shock formation and temperature anisotropy in collisionless magnetic reconnection

    NASA Astrophysics Data System (ADS)

    Higashimori, K.; Hoshino, M.

    2011-12-01

    We perform a two-dimensional simulation by using an electromagnetic hybrid code to study the formation of slow-mode shocks in collisionless magnetic reconnection in low beta plasmas, and we argue that one of important agents of the formation of slow shocks is the ion temperature anisotropy enhanced at the shock downstream region. As magnetic reconnection develops, it is known that the parallel temperature along the magnetic field becomes large in association with the anisotropic PSBL ion beams, and this temperature anisotropy has a tendency to suppress the formation of slow shock. Although preceding studies on magnetic reconnection with kinetic codes have shown such ion temperature anisotropy along the reconnection layer, the direct relation between formation of slow shocks and the ion temperature anisotropy has not been investigated. Based on our simulation result, we found that the slow shock formation is suppressed due to the large temperature anisotropy near the X-type region, but the downstream ion temperature anisotropy relaxes with increasing the distance from the magnetic neutral point. As a result, two pairs of current structures, which are the strong evidence of dissipation of magnetic field in slow shocks, are formed at the distance |x| > 115 λ i from the neutral point.

  17. Magnetic patterning using ion irradiation for highly ordered CoPt alloys with perpendicular anisotropy

    SciTech Connect

    Abes, M.; Venuat, J.; Muller, D.; Carvalho, A.; Schmerber, G.; Beaurepaire, E.; Dinia, A.; Pierron-Bohnes, V.

    2004-12-15

    We used a combination of ion irradiation and e-beam lithography to magnetically pattern an ordered CoPt alloy with strong perpendicular magnetic anisotropy. Ion irradiation disorders the alloy and strongly reduces the magnetic anisotropy. Magnetic force microscopy showed a regular array of 1 {mu}m{sup 2} square dots with perpendicular anisotropy separated by 1 {mu}m large ranges with in-plane anisotropy. This is further confirmed by magnetic measurements, which showed that arrays protected by a 200 nm Pt layer present the same coercive field and the same perpendicular anisotropy as before irradiation. This is promising for applications in magnetic recording technologies.

  18. Soliton collisions in soft magnetic nanotube with uniaxial anisotropy

    NASA Astrophysics Data System (ADS)

    Usov, N. A.

    2016-05-01

    The structure of stable magnetic solitons of various orders in soft magnetic nanotube with uniaxial magnetic anisotropy has been studied using numerical simulation. Solitons of even order are immobile in axially applied magnetic field. Odd solitons show decreased mobility with respect to that of head-to head domain wall. Solitons of various orders can participate in nanotube magnetization reversal process. Various coalescence and decomposition processes in soliton assembly are considered. It is shown that the general magnetization state of magnetic nanotube consists of chains of magnetic solitons of various orders.

  19. Formation of Magnetic Anisotropy by Lithography.

    PubMed

    Kim, Si Nyeon; Nam, Yoon Jae; Kim, Yang Doo; Choi, Jun Woo; Lee, Heon; Lim, Sang Ho

    2016-01-01

    Artificial interface anisotropy is demonstrated in alternating Co/Pt and Co/Pd stripe patterns, providing a means of forming magnetic anisotropy using lithography. In-plane hysteresis loops measured along two principal directions are explained in depth by two competing shape and interface anisotropies, thus confirming the formation of interface anisotropy at the Co/Pt and Co/Pd interfaces of the stripe patterns. The measured interface anisotropy energies, which are in the range of 0.2-0.3 erg/cm(2) for both stripes, are smaller than those observed in conventional multilayers, indicating a decrease in smoothness of the interfaces when formed by lithography. The demonstration of interface anisotropy in the Co/Pt and Co/Pd stripe patterns is of significant practical importance, because this setup makes it possible to form anisotropy using lithography and to modulate its strength by controlling the pattern width. Furthermore, this makes it possible to form more complex interface anisotropy by fabricating two-dimensional patterns. These artificial anisotropies are expected to open up new device applications such as multilevel bits using in-plane magnetoresistive thin-film structures. PMID:27216420

  20. Formation of Magnetic Anisotropy by Lithography

    PubMed Central

    Kim, Si Nyeon; Nam, Yoon Jae; Kim, Yang Doo; Choi, Jun Woo; Lee, Heon; Lim, Sang Ho

    2016-01-01

    Artificial interface anisotropy is demonstrated in alternating Co/Pt and Co/Pd stripe patterns, providing a means of forming magnetic anisotropy using lithography. In-plane hysteresis loops measured along two principal directions are explained in depth by two competing shape and interface anisotropies, thus confirming the formation of interface anisotropy at the Co/Pt and Co/Pd interfaces of the stripe patterns. The measured interface anisotropy energies, which are in the range of 0.2–0.3 erg/cm2 for both stripes, are smaller than those observed in conventional multilayers, indicating a decrease in smoothness of the interfaces when formed by lithography. The demonstration of interface anisotropy in the Co/Pt and Co/Pd stripe patterns is of significant practical importance, because this setup makes it possible to form anisotropy using lithography and to modulate its strength by controlling the pattern width. Furthermore, this makes it possible to form more complex interface anisotropy by fabricating two-dimensional patterns. These artificial anisotropies are expected to open up new device applications such as multilevel bits using in-plane magnetoresistive thin-film structures. PMID:27216420

  1. Single-ion anisotropy and magnetic field response in the spin-ice materials Ho2Ti2O7 and Dy2Ti2O7

    NASA Astrophysics Data System (ADS)

    Tomasello, Bruno; Castelnovo, Claudio; Moessner, Roderich; Quintanilla, Jorge

    2015-10-01

    Motivated by its role as a central pillar of current theories of the dynamics of spin ice in and out of equilibrium, we study the single-ion dynamics of the magnetic rare-earth ions in their local environments, subject to the effective fields set up by the magnetic moments with which they interact. This effective field has a transverse component with respect to the local easy axis of the crystal electric field, which can induce quantum tunneling. We go beyond the projective spin-1/2 picture and use instead the full crystal-field Hamiltonian. We find that the Kramers versus non-Kramers nature, as well as the symmetries of the crystal-field Hamiltonian, result in different perturbative behavior at small fields (≲1 T ), with transverse field effects being more pronounced in Ho2Ti2O7 than in Dy2Ti2O7 . Remarkably, the energy splitting range we find is consistent with time scales extracted from experiments. We also present a study of the static magnetic response, which highlights the anisotropy of the system in the form of an off-diagonal g tensor, and we investigate the effects of thermal fluctuations in the temperature regime of relevance to experiments. We show that there is a narrow but accessible window of experimental parameters where the anisotropic response can be observed.

  2. Interfacial magnetic anisotropy from a 3-dimensional Rashba substrate

    NASA Astrophysics Data System (ADS)

    Li, Junwen; Haney, Paul M.

    2016-07-01

    We study the magnetic anisotropy which arises at the interface between a thin film ferromagnet and a 3-d Rashba material. We use a tight-binding model to describe the bilayer, and the 3-d Rashba material characterized by the spin-orbit strength α and the direction of broken bulk inversion symmetry n ̂ . We find an in-plane uniaxial anisotropy in the z ̂ × n ̂ direction, where z ̂ is the interface normal. For realistic values of α, the uniaxial anisotropy is of a similar order of magnitude as the bulk magnetocrystalline anisotropy. Evaluating the uniaxial anisotropy for a simplified model in 1-d shows that for small band filling, the in-plane easy axis anisotropy scales as α4 and results from a twisted exchange interaction between the spins in the 3-d Rashba material and the ferromagnet. For a ferroelectric 3-d Rashba material, n ̂ can be controlled with an electric field, and we propose that the interfacial magnetic anisotropy could provide a mechanism for electrical control of the magnetic orientation.

  3. Efficient enhancement of magnetic anisotropy by optimizing the ligand-field in a typically tetranuclear dysprosium cluster.

    PubMed

    Liu, Jiang; Chen, Yan-Cong; Jiang, Zhong-Xia; Liu, Jun-Liang; Jia, Jian-Hua; Wang, Long-Fei; Li, Quan-Wen; Tong, Ming-Liang

    2015-05-01

    The perturbation to the ligand field around the lanthanide ion may significantly contribute to the magnetic dynamics of single molecule magnets. This can be demonstrated by two typical Dy4 cluster-based single molecular magnets (SMMs), [Dy4X2(μ3-OH)2(μ-OH)2(2,2-bpt)4(H2O)4]X2·2H2O·4EtOH (X = Cl and Br for and , respectively), which were constructed by using 3,5-bis(pyridin-2-yl)-1,2,4-triazole (2,2-bptH) as the polynuclear-chelating ligand. Alternating-current (ac) magnetic susceptibility measurements show that the energy barriers in complexes and were immensely enhanced by comparing with our previous work due to the optimization of the ligand field around Dy(III) ions. Remarkably, their high thermal active barriers at 190 K () and 197 K () under a zero applied external dc magnetic field are also among the highest within the reported tetranuclear lanthanide-based SMMs. PMID:25837027

  4. Magnetic anisotropy of polycrystalline magnetoferritin investigated by SQUID and electron magnetic resonance

    NASA Astrophysics Data System (ADS)

    Moro, F.; de Miguel, R.; Jenkins, M.; Gómez-Moreno, C.; Sells, D.; Tuna, F.; McInnes, E. J. L.; Lostao, A.; Luis, F.; van Slageren, J.

    2014-06-01

    Magnetoferritin molecules with an average inorganic core diameter of 5.7±1.6 nm and polycrystalline internal structure were investigated by a combination of transmission electron microscopy, magnetic susceptibility, magnetization, and electron magnetic resonance (EMR) experiments. The temperature and frequency dependence of the magnetic susceptibility allowed for the determination of the magnetic anisotropy on an experimental time scale which spans from seconds to nanoseconds. In addition, angle-dependent EMR experiments were carried out for the determination of the nanoparticle symmetry and internal magnetic field. Due to the large surface to volume ratio, the nanoparticles show larger and uniaxial rather than cubic magnetic anisotropies compared to bulk maghemite and magnetite.

  5. Thermal behavior of hard-axis magnetization in noninteracting particles with uniaxial anisotropy

    NASA Astrophysics Data System (ADS)

    Ilievski, F.; Cuchillo, A.; Nunes, W.; Knobel, M.; Ross, C. A.; Vargas, P.

    2009-11-01

    Experimental evidence is presented to support predictions made by an analytical model describing the temperature-dependent behavior of an assembly of noninteracting magnetic nanoparticles with uniaxial anisotropy under an external field. When the applied field is smaller than the anisotropy field of the particles and is oriented perpendicular to the easy axis, a maximum of the magnetization occurs at finite temperature. The theory shows good agreement with measurements of an array of CoCrPt nanoislands with uniaxial anisotropy. Deviations are discussed taking into account the thermal dependencies of the saturation magnetization and the anisotropy of the magnetic material.

  6. Magnetic Anisotropies in Samarium-Cobalt Thin Films

    NASA Astrophysics Data System (ADS)

    Chen, Kailai

    A systemic study of the deposition processes and magnetic properties for the Sm-Co film system has been carried out. Films of Sm-Co system with various magnetic anisotropies have been synthesized through sputter deposition in both crystalline and amorphous phases. The origins of various anisotropies have been studied. Thermallized sputter deposition process control was used to synthesize Fe enriched Sm-Co films with rhombohedral Th_2Zn_{17} type structure. The film exhibited unusually strong textures with the crystallographic c axes of the crystallites aligned in the film plane. A large anisotropy was resulted with easy axis in the film plane. A well defined and large in-the-film-plane anisotropy of exceptionally high value of 3.3 times 10^6 erg/cm^3 has been obtained in the amorphous SmCo films by applying a magnetic field in the film plane during deposition. It was found that the in-the-film-plane anisotropy depended essentially on the applied field and Sm concentration. For films not synthesized through thermallized sputtering, the easy axis of the film could be reoriented through post deposition annealing. In contrast, in-plane easy axes of films synthesized through thermallized sputtering deposition could not be reoriented. A perpendicular anisotropy was also presented in the film synthesized through thermallized sputtering deposition. A large in-plane anisotropy was obtained in films deposited above ambient temperatures. It was concluded that the surface induced short range ordering was the origin of the in-the-film-plane anisotropy observed in amorphous film deposited in the presence of a magnetic field. The formation mechanism was different from that of the short range ordering induced by field annealing. The perpendicular anisotropy was shown to be growth induced. Large in-plane anisotropy in amorphous films was resulted from partial crystallization in the film. Both the formation of growth induced structure and partial crystallization in the film

  7. Direct expressions for magnetic anisotropy constants

    NASA Astrophysics Data System (ADS)

    Miura, Daisuke; Sasaki, Ryo; Sakuma, Akimasa

    2015-11-01

    Direct expressions for the magnetic anisotropy constants are given at a finite temperature from a microscopic viewpoint. The present derivation assumes that the Hamiltonian is a linear function with respect to the magnetization direction. We discuss in detail the first-order anisotropy constant K1 and show that our present results reproduce previous results. We applied our method to Nd2Fe14B compounds and confirmed that the present method can reproduce the temperature dependence of the magnetocrystalline anisotoropy constants K1, K2, and K3 well.

  8. Random Field effects in perpendicular-anisotropy multilayer films

    NASA Astrophysics Data System (ADS)

    Xu, Jian; Silevitch, Daniel; Rosenbaum, Thomas

    With the application of a magnetic field transverse to the magnetic easy axis, randomly-distributed 3D collections of dipole-coupled Ising spins form a realization of the Random-Field Ising Model. Tuning the strength of the site-specific random field, and hence the disorder, via the applied transverse field regulates the domain reversal energetics and hence the macroscopic hysteresis loop. We extend this approach to two dimensions, using sputtered Perpendicular Magnetic Anisotropy (PMA) Co/Pt multilayer thin films. We characterize the coercive fields and hysteresis loops at a series of temperatures and transverse fields.

  9. A comparative study of magnetic anisotropy measurement techniques in relation to rock-magnetic properties

    NASA Astrophysics Data System (ADS)

    Bilardello, Dario; Jackson, Michael J.

    2014-08-01

    Magnetic anisotropy measurements are becoming increasingly common to many studies within the different disciplines of geology, involving sedimentary, igneous and metamorphic rocks. A plethora of techniques exists for measuring magnetic anisotropy of rocks. Some are rapid and non-destructive while others are more labor-intensive or may result in alteration of the magnetic minerals. All, however, have the potential of revealing a wealth of information when measured and interpreted correctly. In broad terms, anisotropy techniques subdivide into measurements of susceptibility, remanence and torque; here we consider the first two of these. Anisotropy of magnetic susceptibility (AMS) is by far the most utilized, and measures composite fabrics. Magnetic susceptibilities in high fields and low temperatures, however, are being increasingly used to isolate the paramagnetic contribution to the fabrics. When distinguishing between fabrics carried by different ferromagnetic phases, or to separate these from the diamagnetic and paramagnetic contributions to the fabric, then remanence anisotropy techniques become necessary. Anisotropies of thermal remanence (ATRMs), of anhysteretic remanence (AARM) and of isothermal remanence (AIRM) are the most common examples. Remanence anisotropy may be measured over the full spectrum of magnetic coercivities or over a targeted range (e.g. partial or ApARM). Moreover, anisotropies may be calculated using only the resolved field-parallel component of the vector, in which case a minimum of six different orientations is necessary to obtain a complete symmetric tensor, or using the three components (full vector) of the measured magnetic vectors (e.g. AvARM), in which case three orthogonal applied magnetizations are the minimum requirement. In this study we utilize a variety of magnetic remanence room temperature techniques to measure remanence anisotropy of selected coarse and finer grained gneiss-granulitic specimens with well-pronounced fabrics

  10. Anisotropy of magnetic susceptibility in alkali feldspar and plagioclase

    NASA Astrophysics Data System (ADS)

    Biedermann, Andrea R.; Pettke, Thomas; Angel, Ross J.; Hirt, Ann M.

    2016-04-01

    Feldspars are the most abundant rock-forming minerals in the Earth's crust, but their magnetic properties have not been rigorously studied. This work focuses on the intrinsic magnetic anisotropy of 31 feldspar samples with various chemical compositions. Because feldspar is often twinned or shows exsolution textures, measurements were performed on twinned and exsolved samples as well as single crystals. The anisotropy is controlled by the diamagnetic susceptibility and displays a consistent orientation of principal susceptibility axes; the most negative or minimum susceptibility is parallel to [010], and the maximum (least negative) is close to the crystallographic [001] axis. However, the magnetic anisotropy is weak when compared to other rock-forming minerals, 1.53 × 10-9 m3 kg-1 at maximum. Therefore, lower abundance minerals, such as augite, hornblende or biotite, often dominate the bulk paramagnetic anisotropy of a rock. Ferromagnetic anisotropy is not significant in most samples. In the few samples that do show ferromagnetic anisotropy, the principal susceptibility directions of the ferromagnetic subfabric do not display a systematic orientation with respect to the feldspar lattice. These results suggest that palaeointensity estimates of the geomagnetic field made on single crystals of feldspar will not be affected by a systematic orientation of the ferromagnetic inclusions within the feldspar lattice.

  11. Anisotropy of magnetic susceptibility in alkali feldspar and plagioclase

    NASA Astrophysics Data System (ADS)

    Biedermann, Andrea R.; Pettke, Thomas; Angel, Ross J.; Hirt, Ann M.

    2016-01-01

    Feldspars are the most abundant rock-forming minerals in the Earth's crust, but their magnetic properties have not been rigorously studied. This work focuses on the intrinsic magnetic anisotropy of 31 feldspar samples with various chemical compositions. Because feldspar is often twinned or shows exsolution textures, measurements were performed on twinned and exsolved samples as well as single crystals. The anisotropy is controlled by the diamagnetic susceptibility and displays a consistent orientation of principal susceptibility axes; the most negative or minimum susceptibility is parallel to [010], and the maximum (least negative) is close to the crystallographic [001] axis. However, the magnetic anisotropy is weak when compared to other rock-forming minerals, 1.53*10-9 m3 kg-1 at maximum. Therefore, lower abundance minerals such as augite, hornblende or biotite often dominate the bulk paramagnetic anisotropy of a rock. Ferromagnetic anisotropy is not significant in most samples. In the few samples that do show ferromagnetic anisotropy, the principal susceptibility directions of the ferromagnetic subfabric do not display a systematic orientation with respect to the feldspar lattice. These results suggest that paleointensity estimates of the geomagnetic field made on single crystals of feldspar will not be affected by a systematic orientation of the ferromagnetic inclusions within the feldspar lattice.

  12. Exotic skyrmion crystals in chiral magnets with compass anisotropy

    PubMed Central

    Chen, J. P.; Zhang, Dan-Wei; Liu, J. -M.

    2016-01-01

    The compass-type anisotropy appears naturally in diverse physical contexts with strong spin-orbit coupling (SOC) such as transition metal oxides and cold atomic gases etc, and it has been receiving substantial attention. Motivated by recent studies and particularly recent experimental observations on helimagnet MnGe, we investigate the critical roles of this compass-type anisotropy in modulating various spin textures of chiral magnets with strong SOC, by Monte Carlo simulations based on a classical Heisenberg spin model with Dzyaloshinsky-Moriya interaction and compass anisotropy. A phase diagram with emergent spin orders in the space of compass anisotropy and out-of-plane magnetic field is presented. In this phase diagram, we propose that a hybrid super-crystal structure consisting of alternating half-skyrmion and half-anti-skyrmion is the possible zero-field ground state of MnGe. The simulated evolution of the spin structure driven by magnetic field is in good accordance with experimental observations on MnGe. Therefore, this Heisenberg spin model successfully captures the main physics responsible for the magnetic structures in MnGe, and the present work may also be instructive to research on the magnetic states in other systems with strong SOC. PMID:27377149

  13. Exotic skyrmion crystals in chiral magnets with compass anisotropy

    NASA Astrophysics Data System (ADS)

    Chen, J. P.; Zhang, Dan-Wei; Liu, J.-M.

    2016-07-01

    The compass-type anisotropy appears naturally in diverse physical contexts with strong spin-orbit coupling (SOC) such as transition metal oxides and cold atomic gases etc, and it has been receiving substantial attention. Motivated by recent studies and particularly recent experimental observations on helimagnet MnGe, we investigate the critical roles of this compass-type anisotropy in modulating various spin textures of chiral magnets with strong SOC, by Monte Carlo simulations based on a classical Heisenberg spin model with Dzyaloshinsky-Moriya interaction and compass anisotropy. A phase diagram with emergent spin orders in the space of compass anisotropy and out-of-plane magnetic field is presented. In this phase diagram, we propose that a hybrid super-crystal structure consisting of alternating half-skyrmion and half-anti-skyrmion is the possible zero-field ground state of MnGe. The simulated evolution of the spin structure driven by magnetic field is in good accordance with experimental observations on MnGe. Therefore, this Heisenberg spin model successfully captures the main physics responsible for the magnetic structures in MnGe, and the present work may also be instructive to research on the magnetic states in other systems with strong SOC.

  14. Exotic skyrmion crystals in chiral magnets with compass anisotropy.

    PubMed

    Chen, J P; Zhang, Dan-Wei; Liu, J-M

    2016-01-01

    The compass-type anisotropy appears naturally in diverse physical contexts with strong spin-orbit coupling (SOC) such as transition metal oxides and cold atomic gases etc, and it has been receiving substantial attention. Motivated by recent studies and particularly recent experimental observations on helimagnet MnGe, we investigate the critical roles of this compass-type anisotropy in modulating various spin textures of chiral magnets with strong SOC, by Monte Carlo simulations based on a classical Heisenberg spin model with Dzyaloshinsky-Moriya interaction and compass anisotropy. A phase diagram with emergent spin orders in the space of compass anisotropy and out-of-plane magnetic field is presented. In this phase diagram, we propose that a hybrid super-crystal structure consisting of alternating half-skyrmion and half-anti-skyrmion is the possible zero-field ground state of MnGe. The simulated evolution of the spin structure driven by magnetic field is in good accordance with experimental observations on MnGe. Therefore, this Heisenberg spin model successfully captures the main physics responsible for the magnetic structures in MnGe, and the present work may also be instructive to research on the magnetic states in other systems with strong SOC. PMID:27377149

  15. Random magnetic anisotropy in isotropic nanocrystalline composite permanent magnets

    NASA Astrophysics Data System (ADS)

    Sato, Suguru; Lee, S. J.; Mitsumata, Chiharu; Yanagihara, Hideto; Kita, Eiji

    2011-04-01

    In this study, the random magnetic anisotropy in isotropic nanocrystalline composite permanent magnets was investigated by means of numerical simulations. The magnetization reversal of randomly oriented hard-soft exchange-coupled grains was simulated using the Landau-Lifshitz-Gilbert equation in which the magnetization in a particular grain is assumed to align in the same direction (single-spin model). The calculations show that the energy product (BH)max of nanocomposite magnets has a peak value 50 MGOe at 6 nm. It is about 80% of that of single-crystal Nd2Fe14B. The coercivity HC exhibits a steep decrease toward smaller grain size, which is the result of the suppression of the random magnetic anisotropy by exchange interaction. Therefore, in isotropic nanocomposite magnets, the enhancement of energy product is limited by the suppression of the random magnetic anisotropy by exchange interaction.

  16. Bubble and skyrmion crystals in frustrated magnets with easy-axis anisotropy

    DOE PAGESBeta

    Hayami, Satoru; Lin, Shi-Zeng; Batista, Cristian D.

    2016-05-12

    We clarify the conditions for the emergence of multiple-Q structures out of lattice and easy-axis spin anisotropy in frustrated magnets. By considering magnets whose exchange interaction has multiple global minima in momentum space, we find that both types of anisotropy stabilize triple-Q orderings. Moderate anisotropy leads to a magnetic field-induced skyrmion crystal, which evolves into a bubble crystal for increasing spatial and spin anisotropy. Finally, the bubble crystal exhibits a quasi-continuous (devil’s staircase) temperature dependent ordering wave-vector, characteristic of the competition between frustrated exchange and strong easy-axis anisotropy.

  17. Bubble and skyrmion crystals in frustrated magnets with easy-axis anisotropy

    NASA Astrophysics Data System (ADS)

    Hayami, Satoru; Lin, Shi-Zeng; Batista, Cristian D.

    2016-05-01

    We clarify the conditions for the emergence of multiple-Q structures out of lattice and easy-axis spin anisotropy in frustrated magnets. By considering magnets whose exchange interaction has multiple global minima in momentum space, we find that both types of anisotropy stabilize triple-Q orderings. Moderate anisotropy leads to a magnetic-field-induced skyrmion crystal, which evolves into a bubble crystal for increasing spatial and spin anisotropy. The bubble crystal exhibits a quasicontinuous (devil's staircase) temperature-dependent ordering wave vector, characteristic of the competition between frustrated exchange and strong easy-axis anisotropy.

  18. Magnetic anisotropy and domain patterning of amorphous films by He-ion irradiation

    SciTech Connect

    McCord, Jeffrey; Gemming, Thomas; Schultz, Ludwig; Fassbender, Juergen; Liedke, Maciej Oskar; Frommberger, Michael; Quandt, Eckhard

    2005-04-18

    The magnetic anisotropy in amorphous soft magnetic FeCoSiB films was modified by He-ion irradiation. A rotation of uniaxial anisotropy depending on the applied field direction in the irradiated areas is observed by magnetometry and complementary domain observation by Kerr microscopy. No significant degradation in magnetic properties relative to the as-deposited state is found from the magnetization loops on nonpatterned films. Using irradiation together with photolithography, the films were treated locally, resulting in 'anisotropy patterned' structures. Complicated periodic domain patterns form due to the locally varying anisotropy distribution. Overall magnetic properties and domain patterns are adjusted.

  19. Magnetic Alignment of Block Copolymer Microdomains by Intrinsic Chain Anisotropy

    NASA Astrophysics Data System (ADS)

    Rokhlenko, Yekaterina; Gopinadhan, Manesh; Osuji, Chinedum O.; Zhang, Kai; O'Hern, Corey S.; Larson, Steven R.; Gopalan, Padma; Majewski, Paweł W.; Yager, Kevin G.

    2015-12-01

    We examine the role of intrinsic chain susceptibility anisotropy in magnetic field directed self-assembly of a block copolymer using in situ x-ray scattering. Alignment of a lamellar mesophase is observed on cooling across the disorder-order transition with the resulting orientational order inversely proportional to the cooling rate. We discuss the origin of the susceptibility anisotropy, Δ χ , that drives alignment and calculate its magnitude using coarse-grained molecular dynamics to sample conformations of surface-tethered chains, finding Δ χ ≈2 ×1 0-8. From field-dependent scattering data, we estimate that grains of ≈1.2 μ m are present during alignment. These results demonstrate that intrinsic anisotropy is sufficient to support strong field-induced mesophase alignment and suggest a versatile strategy for field control of orientational order in block copolymers.

  20. Magnetic alignment of block copolymer microdomains by intrinsic chain anisotropy

    SciTech Connect

    Rokhlenko, Yekaterina; Yager, Kevin G.; Gopinadhan, Manesh; Osuji, Chinedum O.; Zhang, Kai; O'Hern, Corey S.; Larson, Steven R.; Gopalan, Padma; Majewski, Pawel W.

    2015-12-18

    We examine the role of intrinsic chain susceptibility anisotropy in magnetic field directed self-assembly of a block copolymer using in situ x-ray scattering. Alignment of a lamellar mesophase is observed on cooling across the disorder-order transition with the resulting orientational order inversely proportional to the cooling rate. We discuss the origin of the susceptibility anisotropy, Δχ, that drives alignment and calculate its magnitude using coarse-grained molecular dynamics to sample conformations of surface-tethered chains, finding Δχ ≈ 2×10–8. From field-dependent scattering data, we estimate that grains of ≈ 1.2 μm are present during alignment. Furthermore, these results demonstrate that intrinsic anisotropy is sufficient to support strong field-induced mesophase alignment and suggest a versatile strategy for field control of orientational order in block copolymers.

  1. Manipulating the magnetic anisotropy of 3d transition-metal films on Cu(001) and their alloys on Rh(001) by electric field

    NASA Astrophysics Data System (ADS)

    Wang, Zhe; Zhang, Yun; Cao, Juexian

    2013-08-01

    The mechanism of electric field (EF) effects on the magnetocrystalline anisotropy (MCA) in metallic films is investigated by first-principles calculations. Start with a simple system of Fe, Co and Ni monolayer on Cu(001) substrate, we show that the key factor for a large EF-induced MCA modification is that the energy bands cross of d and d (or d and d) is close to the Fermi level. In order to enhance the MCA modification by EF, 4d metal substrates (Rh, Pd) are also discussed. In particular, we find that the magnetization direction can be switched from out-of-plane to in-plane by a small EF for Fe1-xCox alloy films on Rh(001) substrate with x=0.5.

  2. Magnetic Anisotropy in UMn2Ge2

    NASA Astrophysics Data System (ADS)

    Berg, Morgann; de Lozanne, Alex; Baumbach, Ryan; Kim, Jeehoon; Bauer, Eric; Thompson, Joe; Ronning, Filip

    2015-03-01

    UMn2Ge2, a permanent magnet, is a ternary intermetallic compound with a tetragonal crystal structure of type ThCr2Si2 and with space group I4/mmm. Local U and Mn moments in UMn2Ge2 order on their respective sublattices at temperatures near 100 and 380 K, respectively. Previous x-ray diffraction, Kerr rotation angle, and SQUID magnetometry data support the commonly accepted notion that U moments order at low temperature and align Mn moments along the c-axis, introducing anisotropy. Previous results obtained using a multi-mode atomic force microscope in magnetic force microscopy (MFM) mode indeed confirmed that UMn2Ge2 displays uniaxial anisotropy with an easy axis coinciding with the c-axis of the material. However, the branching domains in UMn2Ge2 consistent with uniaxial anisotropy were observed all the way up to room temperature by MFM. This indicates that the effect of uranium moments on the magnetic microstructure of UMn2Ge2 is not limited to low temperatures near the ordering temperature of the uranium sublattice. We further investigate closure domains in the surface of UMn2Ge2 and report on characteristics and signatures of anisotropy revealed by the orientation and periodic structures of closure domains. Supported by NSF Grant DMR-0810119.

  3. Tuning the Magnetic Anisotropy of Single Molecules.

    PubMed

    Heinrich, Benjamin W; Braun, Lukas; Pascual, Jose I; Franke, Katharina J

    2015-06-10

    The magnetism of single atoms and molecules is governed by the atomic scale environment. In general, the reduced symmetry of the surrounding splits the d states and aligns the magnetic moment along certain favorable directions. Here, we show that we can reversibly modify the magnetocrystalline anisotropy by manipulating the environment of single iron(II) porphyrin molecules adsorbed on Pb(111) with the tip of a scanning tunneling microscope. When we decrease the tip-molecule distance, we first observe a small increase followed by an exponential decrease of the axial anisotropy on the molecules. This is in contrast to the monotonous increase observed earlier for the same molecule with an additional axial Cl ligand ( Nat. Phys. 2013 , 9 , 765 ). We ascribe the changes in the anisotropy of both species to a deformation of the molecules in the presence of the attractive force of the tip, which leads to a change in the d level alignment. These experiments demonstrate the feasibility of a precise tuning of the magnetic anisotropy of an individual molecule by mechanical control. PMID:25942560

  4. Strain-assisted magnetization reversal in Co/Ni multilayers with perpendicular magnetic anisotropy.

    PubMed

    Gopman, D B; Dennis, C L; Chen, P J; Iunin, Y L; Finkel, P; Staruch, M; Shull, R D

    2016-01-01

    Multifunctional materials composed of ultrathin magnetic films with perpendicular magnetic anisotropy combined with ferroelectric substrates represent a new approach toward low power, fast, high density spintronics. Here we demonstrate Co/Ni multilayered films with tunable saturation magnetization and perpendicular anisotropy grown directly on ferroelectric PZT [Pb(Zr0.52Ti0.48)O3] substrate plates. Electric fields up to ±2 MV/m expand the PZT by 0.1% and generate at least 0.02% in-plane compression in the Co/Ni multilayered film. Modifying the strain with a voltage can reduce the coercive field by over 30%. We also demonstrate that alternating in-plane tensile and compressive strains (less than 0.01%) can be used to propagate magnetic domain walls. This ability to manipulate high anisotropy magnetic thin films could prove useful for lowering the switching energy for magnetic elements in future voltage-controlled spintronic devices. PMID:27297638

  5. Strain-assisted magnetization reversal in Co/Ni multilayers with perpendicular magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Gopman, D. B.; Dennis, C. L.; Chen, P. J.; Iunin, Y. L.; Finkel, P.; Staruch, M.; Shull, R. D.

    2016-06-01

    Multifunctional materials composed of ultrathin magnetic films with perpendicular magnetic anisotropy combined with ferroelectric substrates represent a new approach toward low power, fast, high density spintronics. Here we demonstrate Co/Ni multilayered films with tunable saturation magnetization and perpendicular anisotropy grown directly on ferroelectric PZT [Pb(Zr0.52Ti0.48)O3] substrate plates. Electric fields up to ±2 MV/m expand the PZT by 0.1% and generate at least 0.02% in-plane compression in the Co/Ni multilayered film. Modifying the strain with a voltage can reduce the coercive field by over 30%. We also demonstrate that alternating in-plane tensile and compressive strains (less than 0.01%) can be used to propagate magnetic domain walls. This ability to manipulate high anisotropy magnetic thin films could prove useful for lowering the switching energy for magnetic elements in future voltage-controlled spintronic devices.

  6. Strain-assisted magnetization reversal in Co/Ni multilayers with perpendicular magnetic anisotropy

    PubMed Central

    Gopman, D. B.; Dennis, C. L.; Chen, P. J.; Iunin, Y. L.; Finkel, P.; Staruch, M.; Shull, R. D.

    2016-01-01

    Multifunctional materials composed of ultrathin magnetic films with perpendicular magnetic anisotropy combined with ferroelectric substrates represent a new approach toward low power, fast, high density spintronics. Here we demonstrate Co/Ni multilayered films with tunable saturation magnetization and perpendicular anisotropy grown directly on ferroelectric PZT [Pb(Zr0.52Ti0.48)O3] substrate plates. Electric fields up to ±2 MV/m expand the PZT by 0.1% and generate at least 0.02% in-plane compression in the Co/Ni multilayered film. Modifying the strain with a voltage can reduce the coercive field by over 30%. We also demonstrate that alternating in-plane tensile and compressive strains (less than 0.01%) can be used to propagate magnetic domain walls. This ability to manipulate high anisotropy magnetic thin films could prove useful for lowering the switching energy for magnetic elements in future voltage-controlled spintronic devices. PMID:27297638

  7. Scale-dependent Normalized Amplitude and Weak Spectral Anisotropy of Magnetic Field Fluctuations in the Solar Wind Turbulence

    NASA Astrophysics Data System (ADS)

    Wang, Xin; Tu, Chuanyi; Marsch, Eckart; He, Jiansen; Wang, Linghua

    2016-01-01

    Turbulence in the solar wind was recently reported to be anisotropic, with the average power spectral index close to -2 when sampling parallel to the local mean magnetic field B0 and close to -5/3 when sampling perpendicular to the local B0. This result was widely considered to be observational evidence for the critical balance theory (CBT), which is derived by making the assumption that the turbulence strength is close to one. However, this basic assumption has not yet been checked carefully with observational data. Here we present for the first time the scale-dependent magnetic-field fluctuation amplitude, which is normalized by the local B0 and evaluated for both parallel and perpendicular sampling directions, using two 30-day intervals of Ulysses data. From our results, the turbulence strength is evaluated as much less than one at small scales in the parallel direction. An even stricter criterion is imposed when selecting the wavelet coefficients for a given sampling direction, so that the time stationarity of the local B0 is better ensured during the local sampling interval. The spectral index for the parallel direction is then found to be -1.75, whereas the spectral index in the perpendicular direction remains close to -1.65. These two new results, namely that the value of the turbulence strength is much less than one in the parallel direction and that the angle dependence of the spectral index is weak, cannot be explained by existing turbulence theories, like CBT, and thus will require new theoretical considerations and promote further observations of solar-wind turbulence.

  8. Ag induced enhancement of perpendicular magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Shern, C. S.; Su, C. W.; Wu, Y. E.; Chen, S. H.

    2001-12-01

    Some interesting magnetic properties were observed after Ag ultrathin films were deposited on Co/Pt(1 1 1). The spin reversal of Co can be prevented when Ag atoms cap Co on Pt(1 1 1). The out-of-plane magnetization has a significant enhancement after annealing at high temperature. The Curie temperature increases from 625 to 710 K as 1 ML of Ag is deposited on 1 ML Co/Pt(1 1 1). The change of surface anisotropy and the formation of a Co-Pt alloy are possible mechanisms for the magnetization enhancement.

  9. Inkjet printing of magnetic materials with aligned anisotropy

    NASA Astrophysics Data System (ADS)

    Song, Han; Spencer, Jeremy; Jander, Albrecht; Nielsen, Jeffrey; Stasiak, James; Kasperchik, Vladek; Dhagat, Pallavi

    2014-05-01

    3-D printing processes, which use drop-on-demand inkjet printheads, have great potential in designing and prototyping magnetic materials. Unlike conventional deposition and lithography, magnetic particles in the printing ink can be aligned by an external magnetic field to achieve both high permeability and low hysteresis losses, enabling prototyping and development of novel magnetic composite materials and components, e.g., for inductor and antennae applications. In this work, we report an inkjet printing technique with magnetic alignment capability. Magnetic films with and without particle alignment are printed, and their magnetic properties are compared. In the alignment-induced hard axis direction, an increase in high frequency permeability and a decrease in hysteresis losses are observed. Our results suggest that unique magnetic structures with arbitrary controllable anisotropy, not feasible otherwise, may be fabricated via inkjet printing.

  10. Impact of magnetic surface anisotropy on the precessional switching of magnetization in Pt-alloy nanofilms

    NASA Astrophysics Data System (ADS)

    Daniel, M.; Arun, R.; Sabareesan, P.

    2012-09-01

    Precessional switching of magnetization in CoPt and FePt nanofilms is investigated by solving the Landau-Lifshitz-Gilbert (LLG) equation analytically and numerically. Switching in these films occurs only above a critical value of the magnetic field, and it further depends on the magnetocrystalline anisotropy and saturation magnetization of the film. The presence of magnetic surface anisotropy in these films reduces the switching time significantly. Also, the switching time in the case of Pt-alloys of Co and Fe is low compared to that in the case of pure Co and Fe films.

  11. On Cosmic Magnetic Fields

    NASA Astrophysics Data System (ADS)

    Florido, E.; Battaner, E.

    2010-12-01

    Magnetic fields are present in all astrophysical media. However, many models and interpretations of observations often ignore them, because magnetic fields are difficult to handle and because they produce complicated morphological features. Here we will comment on the basic intuitive properties, which even if not completely true, provide a first guiding insight on the physics of a particular astrophysical problem. These magnetic properties are not mathematically demonstrated here. How magnetic fields evolve and how they introduce dynamical effects are considered, also including a short comment on General Relativity Magnetohydrodynamics. In a second part we consider some audacious and speculative matters. They are answers to three questions: a) How draw a cube without lifting the pencil from the paper so that when the pen passes through the same side do in the same direction? B) Are MILAGRO anisotropies miraculous? C) Do cosmic magnetic lenses exist?. The last two questions deal with issues related with the interplay between magnetic fields and cosmic ray propagation.

  12. Two-dimensional chiral asymmetry in unidirectional magnetic anisotropy structures

    NASA Astrophysics Data System (ADS)

    Perna, P.; Ajejas, F.; Maccariello, D.; Cuñado, J. L.; Guerrero, R.; Niño, M. A.; Muñoz, M.; Prieto, J. L.; Miranda, R.; Camarero, J.

    2016-05-01

    We investigate the symmetry-breaking effects of magnetic nanostructures that present unidirectional (one-fold) magnetic anisotropy. Angular and field dependent transport and magnetic properties have been studied in two different exchange-biased systems, i.e. ferromagnetic (FM)/ antiferromagnetic (AFM) bilayer and spin-valve structures. We experimentally show the direct relationships between the magnetoresistance (MR) response and the magnetization reversal pathways for any field value and direction. We demonstrate that even though the MR signals are related to different transport phenomena, namely anisotropic magnetoresistance (AMR) and giant magnetoresistance (GMR), chiral asymmetries are found around the magnetization hard-axis direction, in both cases originated from the one-fold symmetry of the interfacial exchange coupling. Our results indicate that the chiral asymmetry of transport and magnetic behaviors are intrinsic of systems with an unidirectional contribution.

  13. Magnetic Anisotropy of Maghemite Nanoparticles Probed by RF Transverse Susceptibility

    NASA Astrophysics Data System (ADS)

    Figueroa, A. I.; Bartolomé, J.; García, L. M.; Bartolomé, F.; Arauzo, A.; Millán, A.; Palacio, F.

    We present radio frequency magnetic transverse susceptibility measurements on γ-Fe2O3 nanoparticles, which yield an estimation of their effective anisotropy constant, Keff as a function of nanoparticle size. The resulting values range from 4 to 8 × 104 erg/cm3, being on the order of the magnetocrystalline anisotropy in bulk maghemite. Keff values increase as the particle diameter increases. Evidences of anisotropy field distribution given by the size distribution in the samples, and interparticle interactions that increase as the particle size increases, are also observed in the TS measurements. The effects of such interparticle interaction overcome those of thermal fluctuations, in contrast with the behavior of other iron oxide particles.

  14. Probing Magnetic Susceptibility Anisotropy of Large-Diameter Armchair Carbon Nanotubes via Magnetic Linear Dichroism Spectroscopy

    NASA Astrophysics Data System (ADS)

    Haroz, Erik; Kono, Junichiro; Searles, Thomas; Tu, Xiaomin; Zheng, Ming; Fagan, Jeffrey; McGill, Stephen; Smirnov, Dmitry

    2012-02-01

    We studied magnetic susceptibility anisotropy, via magnetic linear dichroism spectroscopy, of aqueous suspensions of single-walled carbon nanotubes in high magnetic fields up to 22T using a unique magnet system (Split-Florida Helix magnet). Specifically, we measured magnetic susceptibility anisotropies, δχ, of several armchair species ranging from (5,5)-(13,13) at room temperature over an excitation wavelength range of 400-900 nm. For large diameter armchairs such as (12,12) and (13,13), we have observed some of the strongest alignment in a static magnetic field due to their large diameters. Results will be discussed in comparison with detailed calculations involving the Aharonov-Bohm effect.

  15. Magnetic alignment of block copolymer microdomains by intrinsic chain anisotropy

    DOE PAGESBeta

    Rokhlenko, Yekaterina; Yager, Kevin G.; Gopinadhan, Manesh; Osuji, Chinedum O.; Zhang, Kai; O'Hern, Corey S.; Larson, Steven R.; Gopalan, Padma; Majewski, Pawel W.

    2015-12-18

    We examine the role of intrinsic chain susceptibility anisotropy in magnetic field directed self-assembly of a block copolymer using in situ x-ray scattering. Alignment of a lamellar mesophase is observed on cooling across the disorder-order transition with the resulting orientational order inversely proportional to the cooling rate. We discuss the origin of the susceptibility anisotropy, Δχ, that drives alignment and calculate its magnitude using coarse-grained molecular dynamics to sample conformations of surface-tethered chains, finding Δχ ≈ 2×10–8. From field-dependent scattering data, we estimate that grains of ≈ 1.2 μm are present during alignment. Furthermore, these results demonstrate that intrinsic anisotropymore » is sufficient to support strong field-induced mesophase alignment and suggest a versatile strategy for field control of orientational order in block copolymers.« less

  16. Write operation in MRAM with voltage controlled magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Munira, Kamaram; Pandey, Sumeet; Sandhu, Gurtej

    In non-volatile Magnetic RAM, information is saved in the bistable configuration of the free layer in a magnetic tunnel junction (MTJ). New information can be written to the free layer through magnetic induction (Toggle MRAM) or manipulation of magnetization using electric currents (Spin Transfer Torque MRAM or STT-MRAM). Both of the writing methods suffer from a shortcoming in terms of energy efficiency. This limitation on energy performance is brought about by the need for driving relatively large electrical charge currents through the devices for switching. In STT-MRAM, the nonzero voltage drop across the resistive MTJ leads to significant power dissipation. An energy efficient way to write may be with the assistance of voltage controlled magnetic anisotropy (VCMA), where voltage applied across the MTJ creates an electric field that modulates the interfacial anisotropy between the insulator and free layer. However, VCMA cannot switch the free layer completely by 180 degree rotation of magnetization. It can lower the barrier between the two stable configurations or at best, cancel the barrier, allowing 90 degree rotation. A second mechanism, spin torque or magnetic field, is needed to direct the final switching destination.

  17. Reaching the magnetic anisotropy limit of a 3d metal atom.

    PubMed

    Rau, Ileana G; Baumann, Susanne; Rusponi, Stefano; Donati, Fabio; Stepanow, Sebastian; Gragnaniello, Luca; Dreiser, Jan; Piamonteze, Cinthia; Nolting, Frithjof; Gangopadhyay, Shruba; Albertini, Oliver R; Macfarlane, Roger M; Lutz, Christopher P; Jones, Barbara A; Gambardella, Pietro; Heinrich, Andreas J; Brune, Harald

    2014-05-30

    Designing systems with large magnetic anisotropy is critical to realize nanoscopic magnets. Thus far, the magnetic anisotropy energy per atom in single-molecule magnets and ferromagnetic films remains typically one to two orders of magnitude below the theoretical limit imposed by the atomic spin-orbit interaction. We realized the maximum magnetic anisotropy for a 3d transition metal atom by coordinating a single Co atom to the O site of an MgO(100) surface. Scanning tunneling spectroscopy reveals a record-high zero-field splitting of 58 millielectron volts as well as slow relaxation of the Co atom's magnetization. This striking behavior originates from the dominating axial ligand field at the O adsorption site, which leads to out-of-plane uniaxial anisotropy while preserving the gas-phase orbital moment of Co, as observed with x-ray magnetic circular dichroism. PMID:24812206

  18. Magnetic anisotropy in the frustrated spin-ladder system BiCu2PO6 from magnetostriction in pulsed fields

    NASA Astrophysics Data System (ADS)

    Uchida, Atsuko; Kohama, Yoshimitsu; Wang, Shuang; Jaime, Marcelo; Rüegg, Christian

    2012-02-01

    The spin interactions in BiCu2PO6 have been studied by inelastic neutron scattering, magnetic susceptibility, and numerical calculation. There is strong frustration between magnetic interactions along the ladder leg, JLeg and JNNN, and it has been pointed out that a spin gap persists in this frustrated system. Both Jleg and JNNN are intra-ladder and two-leg ladder is always gapped. Longitudinal magnetostriction (MS) measurements were performed using a fiber optic strain gauge in a 60 T pulsed magnet [1] . Specific heat (Cp) and magnetocaloric effect (MCE) measurements were performed in a 35 T DC magnet. Cp vs T was obtained using both a thermal relaxation time and dual slope techniques. We have in this way determined the (H,T) phase diagram of BiCu2PO6 up to 45 T. The 3D character of phase transitions is suggested by the observation of sharp anomalies in CM and δL/L. Our MCE and MS data provides direct evidence of first-order phase transitions for H//c, while phase transitions for H//a and H//b are characterized as second-order phase transitions. The anisotropic and complex phase boundaries will be discussed. [4pt] [1] Daou R et al., Rev. Sci. Instrum. 81, 033909 (2010).

  19. Modification of crystal anisotropy and enhancement of magnetic moment of Co-doped SnO2 thin films annealed under magnetic field.

    PubMed

    Loya-Mancilla, Sagrario M; Poddar, Pankaj; Das, Raja; Ponce, Hilda E Esparza; Templeton-Olivares, Ivan L; Solis-Canto, Oscar O; Ornelas-Gutierrez, Carlos E; Espinosa-Magaña, Francisco; Olive-Méndez, Sion F

    2014-01-01

    Co-doped SnO2 thin films were grown by sputtering technique on SiO2/Si(001) substrates at room temperature, and then, thermal treatments with and without an applied magnetic field (HTT) were performed in vacuum at 600°C for 20 min. HTT was applied parallel and perpendicular to the substrate surface. Magnetic M(H) measurements reveal the coexistence of a strong antiferromagnetic (AFM) signal and a ferromagnetic (FM) component. The AFM component has a Néel temperature higher than room temperature, the spin axis lies parallel to the substrate surface, and the highest magnetic moment m =7 μB/Co at. is obtained when HTT is applied parallel to the substrate surface. Our results show an enhancement of FM moment per Co(+2) from 0.06 to 0.42 μB/Co at. for the sample on which HTT was applied perpendicular to the surface. The FM order is attributed to the coupling of Co(+2) ions through electrons trapped at the site of oxygen vacancies, as described by the bound magnetic polaron model. Our results suggest that FM order is aligned along [101] direction of Co-doped SnO2 nanocrystals, which is proposed to be the easy magnetization axis. PMID:25489286

  20. Modification of crystal anisotropy and enhancement of magnetic moment of Co-doped SnO2 thin films annealed under magnetic field

    PubMed Central

    2014-01-01

    Co-doped SnO2 thin films were grown by sputtering technique on SiO2/Si(001) substrates at room temperature, and then, thermal treatments with and without an applied magnetic field (HTT) were performed in vacuum at 600°C for 20 min. HTT was applied parallel and perpendicular to the substrate surface. Magnetic M(H) measurements reveal the coexistence of a strong antiferromagnetic (AFM) signal and a ferromagnetic (FM) component. The AFM component has a Néel temperature higher than room temperature, the spin axis lies parallel to the substrate surface, and the highest magnetic moment m =7 μB/Co at. is obtained when HTT is applied parallel to the substrate surface. Our results show an enhancement of FM moment per Co+2 from 0.06 to 0.42 μB/Co at. for the sample on which HTT was applied perpendicular to the surface. The FM order is attributed to the coupling of Co+2 ions through electrons trapped at the site of oxygen vacancies, as described by the bound magnetic polaron model. Our results suggest that FM order is aligned along [101] direction of Co-doped SnO2 nanocrystals, which is proposed to be the easy magnetization axis. PMID:25489286

  1. Electroplated FeNi ring cores for fluxgates with field induced radial anisotropy

    NASA Astrophysics Data System (ADS)

    Butta, M.; Ripka, P.; Janosek, M.; Pribil, M.

    2015-05-01

    Being able to control the anisotropy of a magnetic core plays an important role in the development of a fluxgate sensor. Our aim is to induce anisotropy orthogonal to the direction of excitation because it generates a stable, low-noise fluxgate, as cited in the literature. In this paper, we present an original method for electroplating a ring core for a fluxgate with built-in radial anisotropy by performing the electroplating in a radial field produced by a novel yoke. The results show that the resulting anisotropy is homogeneously radial and makes the magnetization rotate, avoiding domain wall movement for low excitation fields.

  2. Giant induced magnetic anisotropy In strain annealed Co-based nanocomposite alloys

    NASA Astrophysics Data System (ADS)

    Kernion, Samuel J.; Ohodnicki, Paul. R.; Grossmann, Jane; Leary, Alex; Shen, Shen; Keylin, Vladimir; Huth, Joseph F.; Horwath, John; Lucas, Matthew S.; McHenry, Michael E.

    2012-09-01

    Low loss switching of soft magnetic materials at high frequencies benefits from tuning the induced anisotropy. We show induced anisotropies, Ku, as large as 1.89×104 J /m3, developed by strain annealing of Co-rich nanocomposite alloys. Crystalline phases in this alloy system have large negative magnetostrictive coefficients, leading to anisotropy fields per unit stress over twice those developed in FINEMET. Tunable permeability and reduced thicknesses achieved in this process can mitigate eddy-current losses. Giant induced magnetic anisotropies are discussed in light of models for the micromechanisms of amorphous metal deformation, stress-assisted transformations in the crystallites, and directional pair ordering.

  3. Measurement of the magnetic anisotropy energy constants for magneto-optical recording media

    NASA Technical Reports Server (NTRS)

    Hajjar, R. A.; Wu, T. H.; Mansuripur, M.

    1992-01-01

    Measurement of the magneto-optical polar Kerr effect is performed on rare earth-transition metal (RE-TM) amorphous films using in-plane fields. From this measurement and the measurement of the saturation magnetization using a vibrating sample magnetometer (VSM), the magnetic anisotropy constants are determined. The temperature dependence is presented of the magnetic anisotropy in the range of -175 to 175 C. The results show a dip in the anisotropy near magnetic compensation. This anomaly is explained based on the finite exchange coupling between the rare earth and transition metal subnetworks.

  4. Transfer matrices for magnetized CMB anisotropies

    SciTech Connect

    Giovannini, Massimo

    2006-05-15

    Large-scale magnetic fields can affect scalar cosmological perturbations whose evolution is described in the conformally Newtonian gauge and within the tight coupling approximation. The magnetized curvature perturbations present after matter-radiation equality (and prior to decoupling) are computed in terms of an appropriate transfer matrix allowing a general estimate of the Sachs-Wolfe plateau. From the observation that CMB initial conditions should be (predominantly) adiabatic, the contribution of the magnetic field intensity can be constrained.

  5. In-plane electric field controlled perpendicular magnetic anisotropy in an FePt/[Pb(Mg1/3Nb2/3)O3]0.7–(PbTiO3)0.3 heterostructure

    NASA Astrophysics Data System (ADS)

    Guo, Qi; Xu, Xiaoguang; Feng, Julong; Liu, Pengfei; Wu, Yong; Ma, Li; Zhou, Shiming; Miao, Jun; Jiang, Yong

    2016-06-01

    We report the in-plane electric field controlled perpendicular magnetic anisotropy of L10-FePt films deposited on polarized [Pb(Mg1/3Nb2/3)O3]0.7–(PbTiO3)0.3 single crystal substrates. The out-of-plane coercivity (H c⊥) of FePt films exhibits a regular response to the in-plane electric field applied on substrates. The experimental change of H c⊥ is approximately 21.3% with the electric field varying from ‑10 to 10 kV/cm. The magnetization direction can be controlled by switching the electric field. The remanence of FePt films can also be manipulated by the electric field, so that a “W”-shaped sawtooth magnetic signal can be generated by a sawtooth electric field.

  6. Inkjet printed superparamagnetic polymer composite hemispheres with programmed magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Ergeneman, Olgaç; Peters, Christian; Gullo, Maurizio R.; Jacot-Descombes, Loïc; Gervasoni, Simone; Özkale, Berna; Fatio, Philipe; Cadarso, Victor J.; Mastrangeli, Massimo; Pané, Salvador; Brugger, Jürgen; Hierold, Christofer; Nelson, Bradley J.

    2014-08-01

    We present the fabrication and characterization of large arrays of inkjet-printed superparamagnetic polymer composite (SPMPC) hemispherical microstructures. SPMPCs are appealing for applications in microsystems and nanorobotics due to the added functionality of polymers and the significant magnetic attributes of embedded nanostructures. SPMPC-based microarchitectures can be used to perform different functions wirelessly in various media (e.g. water, solvents) using external magnetic fields: handling and assembling small objects, delivering drugs or biomass, or sensing specific physical or chemical changes. In this work superparamagnetic magnetite nanoparticles are dispersed in SU-8 to form magnetic hemispheres. Magnetically anisotropic hemispheres as well as standard SPMPC hemispheres are fabricated. Magnetic anisotropy is programmed by applying a magnetic field during curing. The distribution of nanoparticles inside the polymer matrix and magnetic characteristics of the SPMPC are investigated. Magnetic manipulation of hemispheres is demonstrated at liquid-liquid interfaces. Different assembly strategies to form lines or geometric shapes from hemispheres as well as their independent dynamic control are demonstrated. Finally, a two-interface assembly strategy is demonstrated to assemble hemispheres into complete spheres for advanced self-assembly tasks.We present the fabrication and characterization of large arrays of inkjet-printed superparamagnetic polymer composite (SPMPC) hemispherical microstructures. SPMPCs are appealing for applications in microsystems and nanorobotics due to the added functionality of polymers and the significant magnetic attributes of embedded nanostructures. SPMPC-based microarchitectures can be used to perform different functions wirelessly in various media (e.g. water, solvents) using external magnetic fields: handling and assembling small objects, delivering drugs or biomass, or sensing specific physical or chemical changes. In this

  7. Manipulating magnetic anisotropy and ultrafast spin dynamics of magnetic nanostructures

    NASA Astrophysics Data System (ADS)

    Cheng, Zhao-Hua; He, Wei; Zhang, Xiang-Qun; Sun, Da-Li; Du, Hai-Feng; Wu, Qiong; Ye, Jun; Fang, Ya-Peng; Liu, Hao-Liang

    2015-07-01

    We present our extensive research into magnetic anisotropy. We tuned the terrace width of Si(111) substrate by a novel method: varying the direction of heating current and consequently manipulating the magnetic anisotropy of magnetic structures on the stepped substrate by decorating its atomic steps. Laser-induced ultrafast demagnetization of a CoFeB/MgO/CoFeB magnetic tunneling junction was explored by the time-resolved magneto-optical Kerr effect (TR-MOKE) for both the parallel state (P state) and the antiparallel state (AP state) of the magnetizations between two magnetic layers. It was observed that the demagnetization time is shorter and the magnitude of demagnetization is larger in the AP state than those in the P state. These behaviors are attributed to the ultrafast spin transfer between two CoFeB layers via the tunneling of hot electrons through the MgO barrier. Our observation indicates that ultrafast demagnetization can be engineered by the hot electron tunneling current. This opens the door to manipulate the ultrafast spin current in magnetic tunneling junctions. Furthermore, an all-optical TR-MOKE technique provides the flexibility for exploring the nonlinear magnetization dynamics in ferromagnetic materials, especially with metallic materials. Project supported by the National Basic Research Program of China (Grant Nos. 2015CB921403, 2011CB921801, and 2012CB933101) and the National Natural Science Foundation of China (Grant Nos. 51427801, 11374350, 51201179, and 11274361).

  8. Study of YBCO tape anisotropy as a function of field, field orientation and operating temperature

    SciTech Connect

    Lombardo, v.; Barzi, E.; Turrioni, D.; Zlobin, A.V.

    2011-06-01

    Superconducting magnets with magnetic fields above 20 T will be needed for a Muon Collider and possible LHC energy upgrade. This field level exceeds the possibilities of traditional Low Temperature Superconductors (LTS) such as Nb{sub 3}Sn and Nb{sub 3}Al. Presently the use of high field high temperature superconductors (HTS) is the only option available for achieving such field levels. Commercially available YBCO comes in tapes and shows noticeable anisotropy with respect to field orientation, which needs to be accounted for during magnet design. In the present work, critical current test results are presented for YBCO tape manufactured by Bruker. Short sample measurements results are presented up to 14 T, assessing the level of anisotropy as a function of field, field orientation and operating temperature.

  9. Second order anisotropy contribution in perpendicular magnetic tunnel junctions

    PubMed Central

    Timopheev, A. A.; Sousa, R.; Chshiev, M.; Nguyen, H. T.; Dieny, B.

    2016-01-01

    Hard-axis magnetoresistance loops were measured on perpendicular magnetic tunnel junction pillars of diameter ranging from 50 to 150 nm. By fitting these loops to an analytical model, the effective anisotropy fields in both free and reference layers were derived and their variations in temperature range between 340 K and 5 K were determined. It is found that a second-order anisotropy term of the form −K2cos4θ must be added to the conventional uniaxial –K1cos2θ term to explain the experimental data. This higher order contribution exists both in the free and reference layers. At T = 300 K, the estimated −K2/K1 ratios are 0.1 and 0.24 for the free and reference layers, respectively. The ratio is more than doubled at low temperatures changing the ground state of the reference layer from “easy-axis” to “easy-cone” regime. The easy-cone regime has clear signatures in the shape of the hard-axis magnetoresistance loops. The existence of this higher order anisotropy was also confirmed by ferromagnetic resonance experiments on FeCoB/MgO sheet films. It is of interfacial nature and is believed to be due to spatial fluctuations at the nanoscale of the first order anisotropy parameter at the FeCoB/MgO interface. PMID:27246631

  10. Second order anisotropy contribution in perpendicular magnetic tunnel junctions.

    PubMed

    Timopheev, A A; Sousa, R; Chshiev, M; Nguyen, H T; Dieny, B

    2016-01-01

    Hard-axis magnetoresistance loops were measured on perpendicular magnetic tunnel junction pillars of diameter ranging from 50 to 150 nm. By fitting these loops to an analytical model, the effective anisotropy fields in both free and reference layers were derived and their variations in temperature range between 340 K and 5 K were determined. It is found that a second-order anisotropy term of the form -K2cos(4)θ must be added to the conventional uniaxial -K1cos(2)θ term to explain the experimental data. This higher order contribution exists both in the free and reference layers. At T = 300 K, the estimated -K2/K1 ratios are 0.1 and 0.24 for the free and reference layers, respectively. The ratio is more than doubled at low temperatures changing the ground state of the reference layer from "easy-axis" to "easy-cone" regime. The easy-cone regime has clear signatures in the shape of the hard-axis magnetoresistance loops. The existence of this higher order anisotropy was also confirmed by ferromagnetic resonance experiments on FeCoB/MgO sheet films. It is of interfacial nature and is believed to be due to spatial fluctuations at the nanoscale of the first order anisotropy parameter at the FeCoB/MgO interface. PMID:27246631

  11. Second order anisotropy contribution in perpendicular magnetic tunnel junctions

    NASA Astrophysics Data System (ADS)

    Timopheev, A. A.; Sousa, R.; Chshiev, M.; Nguyen, H. T.; Dieny, B.

    2016-06-01

    Hard-axis magnetoresistance loops were measured on perpendicular magnetic tunnel junction pillars of diameter ranging from 50 to 150 nm. By fitting these loops to an analytical model, the effective anisotropy fields in both free and reference layers were derived and their variations in temperature range between 340 K and 5 K were determined. It is found that a second-order anisotropy term of the form ‑K2cos4θ must be added to the conventional uniaxial –K1cos2θ term to explain the experimental data. This higher order contribution exists both in the free and reference layers. At T = 300 K, the estimated ‑K2/K1 ratios are 0.1 and 0.24 for the free and reference layers, respectively. The ratio is more than doubled at low temperatures changing the ground state of the reference layer from “easy-axis” to “easy-cone” regime. The easy-cone regime has clear signatures in the shape of the hard-axis magnetoresistance loops. The existence of this higher order anisotropy was also confirmed by ferromagnetic resonance experiments on FeCoB/MgO sheet films. It is of interfacial nature and is believed to be due to spatial fluctuations at the nanoscale of the first order anisotropy parameter at the FeCoB/MgO interface.

  12. Field dependence of the residual-resistivity anisotropy in sodium and potassium

    NASA Astrophysics Data System (ADS)

    Huberman, M.; Overhauser, A. W.

    1985-01-01

    Recent measurements of the low-field, induced torque in sodium and potassium by Elliott and Datars show that the resistivity anisotropy increases with increasing magnetic field. The zero-field resistivity anisotropy, unexpected for cubic symmetry, is explained by the charge-density-wave (CDW) structure. Due to the wave-function mixing caused by the CDW potential, the momentum transfer (by isotropic impurities) is much larger for electrons near the CDW energy gap. This is modeled by an anisotropic relaxation time in k--> space. The Boltzmann transport equation in a magnetic field can then be solved exactly. The computed resistivity anisotropy is higher for ωcτ>1 compared with its zero-field value. The effect of the magnetic field is to ``stir'' the electron distribution f(k-->) this feeds electrons into the region of rapid relaxation and thereby increases the resistivity anisotropy.

  13. Paleomagnetic, Anisotropy of Magnetic Susceptibility, and 40AR/39AR Data from the Cienega Volcano, Cerros del Rio Volcanic Field, New Mexico

    NASA Astrophysics Data System (ADS)

    Foucher, M. S.; Petronis, M. S.; Lindline, J.; Van Wyk de Vries, B.

    2012-12-01

    Cinder cone eruptions are typically interpreted to have formed by the ascension of magma through a simple conduit. Recent field work and laboratory studies on different excavated volcanoes around the world suggest that magma transport within cinder cones can involve a complex system of feeder geometries. We studied the Cienega volcano, a cinder cone in the Cerros del Rio volcanic field, northern New Mexico, in order to better understand the complexity and the evolution of volcanic plumbing systems in the development of cinder cone volcanoes. We hypothesized that cinder cone plumbing systems are inherently complex and involve numerous feeder geometries (e.g. dikes, sills) and flow patterns both towards and away from the central vent complex. The Cienega volcano comprises tephra fall deposits as well as several vents, multiple intrusions, and numerous lava flow sequences. We inspected the magmatic plumbing system using different laboratory methods including paleomagnetic, anisotropy of magnetic susceptibility (AMS), rock magnetic and thin section studies. We collected samples across each outcrop of the feeder system. The dikes are olivine porphyritic basalts with major clinopyroxene, calcic plagioclase feldspar, magnetite, and xenocrystic quartz. Most samples display a trachytic texture with plagioclase crystals showing a preferred orientation parallel to the dike margins. The magnetic information is held predominantly by a cubic phase magnetite with a low- to moderate-Ti composition of Single or Pseudo-Single Domain grains. The AMS results show various flow directions. Three of six dikes yielded magma flow directions away from the vent. The other dikes showed both a subvertical flow, which corresponds to the typical movement of magma in a dike originating from a deeper crustal level, and a downward flow direction. We concluded that magma initially flowed upward from the magma chamber until it encountered flow resistance. At this structural level (the current

  14. Anisotropy of hyperfine interactions as a tool for interpretation of NMR spectra in magnetic materials.

    PubMed

    Chlan, V; Stěpánková, H; Rezníček, R; Novák, P

    2011-07-01

    Approach for interpretation of nuclear magnetic resonance (NMR) spectra in magnetic materials is presented, consisting in employing the anisotropy of hyperfine interaction. The anisotropic parts of hyperfine magnetic fields on (57)Fe nuclei are calculated ab initio for a model example of lithium ferrite and utilized to assign the experimental NMR spectral lines to iron sites in the crystal structure. PMID:21536415

  15. Quantum theory of the anisotropy of the magnetic properties of ferrimagnetic holmium iron garnet single crystals.

    PubMed

    Yang, Jiehui; Ma, Shengcan; Xu, You

    2009-03-01

    The pronounced anisotropy of the magnetization caused by the Ho(3+) ions in the ferrimagnetic holmium iron garnet has been investigated based on quantum theory. The strong anisotropy of the magnetization of the Ho(3+) ions originates mainly from the effect of the crystal field upon the Ho(3+) ions and the anisotropic Ho(3+)-Fe(3+) superexchange interaction. Following the expression of the Yb(3+)-Fe(3+) exchange interaction used by Alben, the anisotropy of the Ho(3+)-Fe(3+) exchange interaction is defined by three principal values of the exchange tensor G. Because the six Ho(3+) sublattices are magnetically non-equivalent, we calculate the magnetic quantities of the Ho(3+) at the six sublattices and compare the average value of the so-obtained six quantities with the measured values. The calculated results are in good agreement with experiments. An interpretation on the anisotropy of the magnetic properties of HoIG is given. PMID:21817410

  16. Carrier-dependent magnetic anisotropy of Gd-adsorbed graphene

    NASA Astrophysics Data System (ADS)

    Lu, Yuan; Zhou, Tie-ge; Shao, Bin; Zuo, Xu; Feng, Min

    2016-05-01

    Using first-principles calculation based on density functional theory, we study the magnetic anisotropy of Gd-adsorbed graphene and its dependence on carrier accumulation. We show that carrier accumulation not only impacts the magnitude of magnetic anisotropy but also switches its sign. Hole accumulation enhances the perpendicular anisotropy up to ˜16 meV per Gd atom, while electron accumulation switches the anisotropy from perpendicular to in-plane direction. Moreover, we find that the first order perturbation of spin-orbit coupling interaction induces a pseudo-gap at Γ for the perpendicular magnetization, which leads to the the anomalous magnetic anisotropy for the neutral composite. Our findings pave the way for magneto-electric materials based on rare-earth-decorated graphene for voltage-controlled spintronics.

  17. Effects of domain, grain, and magnetic anisotropy distributions on magnetic permeability: Monte-Carlo approach

    SciTech Connect

    Chun, Jaehun; Jones, Anthony M.; McCloy, John S.

    2012-07-23

    Existing approaches for prediction of the tensor permeability of polycrystalline ferrites may not provide reasonable estimates of demagnetized permeability below the spin resonance (i.e., low-field loss region) or in cases of partial magnetization. We propose an approach which solves the coupled Landau-Lifshitz-Gilbert equation for the dynamic magnetic fields including the minimization of free energy to determine the equilibrium magnetization direction. Unlike previous models, we employ a Monte-Carlo approach to easily calculate the (ensemble) averages of permeability over various domain/grain structures and magnetic anisotropy conditions. Material differences, such as those resulting from different preparation methods, are expressed by using probability density functions (p.d.f.) for anisotropy angle (easy axis angle), grain demagnetization factor (ng), and domain demagnetization factor (nd). Effects on the permeability tensor of grain and domain demagnetization factors and anisotropy field relative to saturation magnetization are discussed for the partially magnetized states for polycrystalline ferrites. It is found that the grain structure (i.e., grain demagnetization distribution) has a smaller effect on the frequency dependent permeability than does the same distribution of domains (i.e., domain demagnetization distribution).

  18. Anomalous enhancement in interfacial perpendicular magnetic anisotropy through uphill diffusion

    NASA Astrophysics Data System (ADS)

    Das, Tanmay; Kulkarni, Prabhanjan D.; Purandare, S. C.; Barshilia, Harish C.; Bhattacharyya, Somnath; Chowdhury, Prasanta

    2014-06-01

    We observed interfacial chemical sharpening due to uphill diffusion in post annealed ultrathin multilayer stack of Co and Pt, which leads to enhanced interfacial perpendicular magnetic anisotropy (PMA). This is surprising as these elements are considered as perfectly miscible. This chemical sharpening was confirmed through quantitative energy dispersive x-ray (EDX) spectroscopy and intensity distribution of images taken on high angle annular dark field (HAADF) detector in Scanning Transmission Electron Microscopic (STEM) mode. This observation demonstrates an evidence of miscibility gap in ultrathin coherent Co/Pt multilayer stacks.

  19. Magnetic anisotropy in rapidly quenched amorphous glass-coated nanowires

    NASA Astrophysics Data System (ADS)

    Óvári, T.-A.; Rotărescu, C.; Atițoaie, A.; Corodeanu, S.; Lupu, N.; Chiriac, H.

    2016-07-01

    Results on the roles played by the magnetoelastic and magnetostatic anisotropy terms in the magnetic behavior of glass-coated magnetostrictive amorphous nanowires prepared by means of rapid solidification are reported. Their contributions have been analyzed both experimentally, through hysteresis loop measurements, and theoretically, using micromagnetic simulations. All the investigated samples exhibit a magnetically bistable behavior, characterized by a single-step magnetization reversal when the applied field reaches a critical threshold value, called switching field. The combined interpretation of the experimental and theoretical data allows one to understand the effect of the magnetoelastic term on the value of the switching field, on one hand, and the effect of the magnetostatic term on the nucleation mechanism on the other, both with an essential impact on the characteristics of the nanowires' magnetic bistability. The results are crucial for understanding the basic magnetic properties of these novel rapidly solidified ultrathin magnetic wires, as well as for tailoring their properties according to the specific requirements of various sensing applications.

  20. Interplay between magnetic anisotropy and vibron-assisted tunneling in a single-molecule magnet transistor

    NASA Astrophysics Data System (ADS)

    Park, Kyungwha; McCaskey, Alexander; Yamamoto, Yoh; Warnock, Michael; Burzuri, Enrique; van der Zant, Herre

    2015-03-01

    Molecules trapped in single-molecule devices vibrate with discrete frequencies characteristic to the molecules, and the molecular vibrations can couple to electronic charge and/or spin degrees of freedom. For a significant electron-vibron coupling, electrons may tunnel via the vibrational excitations unique to the molecules. Recently, electron transport via individual anisotropic magnetic molecules (referred to as single-molecule magnets) has been observed in single-molecule transistors. A single-molecule magnet has a large spin moment and a large magnetic anisotropy barrier. So far, studies of electron-vibron coupling effects in single-molecule devices, are mainly for isotropic molecules. Here we investigate how the electron-vibron coupling influences electron transport via a single-molecule magnet Fe4, by using a model Hamiltonian with parameter values obtained from density-functional theory (arXiv:1411.2677). We show that the magnetic anisotropy of the Fe4 induces new features in vibrational conductance peaks and creates vibrational satellite peaks. The main and satellite peak heights have a strong, unusual dependence on the direction and magnitude of applied magnetic field, because the magnetic anisotropy barrier is comparable to vibrational energies. Funding from NSF DMR-1206354, EU FP7 program project 618082 ACMOL, advanced ERC grant (Mols@Mols). Computer resources from SDSC Trestles under DMR060009N and VT ARC.

  1. Direct observation of an anisotropic in-plane residual stress induced by B addition as an origin of high magnetic anisotropy field of Ru/FeCoB film

    NASA Astrophysics Data System (ADS)

    Hirata, Ken-ichiro; Gomi, Shunsuke; Mashiko, Yasuhiro; Nakagawa, Shigeki

    2010-05-01

    Although boron-free FeCo films prepared on a Ru underlayer exhibits isotropic in-plane magnetic property, boron added FeCoB films prepared on Ru underlayer revealed large in-plane magnetic anisotropy with a high anisotropy field of 500 Oe. The effect of boron addition on the in-plane anisotropic residual stress in FeCoB film was investigated using sin2 ψ method of x-ray diffraction analysis. Large isotropic compressive stress was observed in Ru/FeCo film. In contrast, anisotropic in-plane residual stress was observed in Ru/FeCoB film. The compressive stress along the easy axis of Ru/FeCoB film is released more than that along the hard axis. Such anisotropic residual stress is regarded as an origin of the in-plane magnetic anisotropy through inverse magnetostriction effect. Owing to the configuration of the facing targets sputtering system, boron atoms are sputtered and deposited anisotropically, and so they penetrate FeCo crystals and release the compressive stress along the incidence direction.

  2. Direct observation of an anisotropic in-plane residual stress induced by B addition as an origin of high magnetic anisotropy field of Ru/FeCoB film

    SciTech Connect

    Hirata, Ken-ichiro; Gomi, Shunsuke; Mashiko, Yasuhiro; Nakagawa, Shigeki

    2010-05-15

    Although boron-free FeCo films prepared on a Ru underlayer exhibits isotropic in-plane magnetic property, boron added FeCoB films prepared on Ru underlayer revealed large in-plane magnetic anisotropy with a high anisotropy field of 500 Oe. The effect of boron addition on the in-plane anisotropic residual stress in FeCoB film was investigated using sin{sup 2} {psi} method of x-ray diffraction analysis. Large isotropic compressive stress was observed in Ru/FeCo film. In contrast, anisotropic in-plane residual stress was observed in Ru/FeCoB film. The compressive stress along the easy axis of Ru/FeCoB film is released more than that along the hard axis. Such anisotropic residual stress is regarded as an origin of the in-plane magnetic anisotropy through inverse magnetostriction effect. Owing to the configuration of the facing targets sputtering system, boron atoms are sputtered and deposited anisotropically, and so they penetrate FeCo crystals and release the compressive stress along the incidence direction.

  3. Tuning the magnetic anisotropy in single-layer crystal structures

    NASA Astrophysics Data System (ADS)

    Torun, E.; Sahin, H.; Bacaksiz, C.; Senger, R. T.; Peeters, F. M.

    2015-09-01

    The effect of an applied electric field and the effect of charging are investigated on the magnetic anisotropy (MA) of various stable two-dimensional (2D) crystals such as graphene, FeCl2, graphone, fluorographene, and MoTe2 using first-principles calculations. We found that the magnetocrystalline anisotropy energy of Co-on-graphene and Os-doped-MoTe2 systems change linearly with electric field, opening the possibility of electric field tuning MA of these compounds. In addition, charging can rotate the easy-axis direction of Co-on-graphene and Os-doped-MoTe2 systems from the out-of-plane (in-plane) to in-plane (out-of-plane) direction. The tunable MA of the studied materials is crucial for nanoscale electronic technologies such as data storage and spintronics devices. Our results show that controlling the MA of the mentioned 2D crystal structures can be realized in various ways, and this can lead to the emergence of a wide range of potential applications where the tuning and switching of magnetic functionalities are important.

  4. Transition Ion Strikes Back: Large Magnetic Susceptibility Anisotropy in Cobalt(II) Clathrochelates.

    PubMed

    Novikov, Valentin V; Pavlov, Alexander A; Belov, Alexander S; Vologzhanina, Anna V; Savitsky, Anton; Voloshin, Yan Z

    2014-11-01

    Transition-metal complexes are rarely considered as paramagnetic tags for NMR spectroscopy due to them generally having relatively low magnetic anisotropy. Here we report cobalt(II) cage complexes with the largest (among the transition-metal complexes) axial anisotropy of magnetic susceptibility, reaching as high as 12.6 × 10(-32) m(3) at room temperature. This remarkable anisotropy, which results from an unusual trigonal prismatic geometry of the complexes and translates into large negative value of the zero-field splitting energy, is high enough to promote reliable paramagnetic pseudocontact shifts at the distance beyond 2 nm. Our finding paves the way toward the applications of cobalt(II) clathrochelates as future paramagnetic tags. Given the incredible stability and functionalization versatility of clathrochelates, the fine-tuning of the caging ligand may lead to new chemically stable mononuclear single-molecule magnets, for which magnetic anisotropy is of importance. PMID:26278750

  5. Phase diagram of a three-dimensional antiferromagnet with random magnetic anisotropy.

    PubMed

    Perez, Felio A; Borisov, Pavel; Johnson, Trent A; Stanescu, Tudor D; Trappen, Robbyn; Holcomb, Mikel B; Lederman, David; Fitzsimmons, M R; Aczel, Adam A; Hong, Tao

    2015-03-01

    Three-dimensional antiferromagnets with random magnetic anisotropy (RMA) that have been experimentally studied to date have competing two-dimensional and three-dimensional exchange interactions which can obscure the authentic effects of RMA. The magnetic phase diagram of Fe_{x}Ni_{1-x}F_{2} epitaxial thin films with true random single-ion anisotropy was deduced from magnetometry and neutron scattering measurements and analyzed using mean-field theory. Regions with uniaxial, oblique, and easy-plane anisotropies were identified. A RMA-induced glass region was discovered where a Griffiths-like breakdown of long-range spin order occurs. PMID:25793845

  6. Phase Diagram of a Three-Dimensional Antiferromagnet with Random Magnetic Anisotropy

    SciTech Connect

    Perez, Felio A.; Borisov, Pavel; Johnson, Trent A.; Stanescu, Tudor D.; Trappen, Robbyn; Holcomb, Mikel B.; Lederman, David; Fitzsimmons, M. R.; Aczel, Adam A.; Hong, Tao

    2015-03-04

    Three-dimensional (3D) antiferromagnets with random magnetic anisotropy (RMA) that were experimentally studied to date have competing two-dimensional and three-dimensional exchange interactions which can obscure the authentic effects of RMA. The magnetic phase diagram of FexNi1-xF2 epitaxial thin films with true random single-ion anisotropy was deduced from magnetometry and neutron scattering measurements and analyzed using mean field theory. Regions with uniaxial, oblique and easy plane anisotropies were identified. A RMA-induced glass region was discovered where a Griffiths-like breakdown of long-range spin order occurs.

  7. Phase Diagram of a Three-Dimensional Antiferromagnet with Random Magnetic Anisotropy

    DOE PAGESBeta

    Perez, Felio A.; Borisov, Pavel; Johnson, Trent A.; Stanescu, Tudor D.; Trappen, Robbyn; Holcomb, Mikel B.; Lederman, David; Fitzsimmons, M. R.; Aczel, Adam A.; Hong, Tao

    2015-03-04

    Three-dimensional (3D) antiferromagnets with random magnetic anisotropy (RMA) that were experimentally studied to date have competing two-dimensional and three-dimensional exchange interactions which can obscure the authentic effects of RMA. The magnetic phase diagram of FexNi1-xF2 epitaxial thin films with true random single-ion anisotropy was deduced from magnetometry and neutron scattering measurements and analyzed using mean field theory. Regions with uniaxial, oblique and easy plane anisotropies were identified. A RMA-induced glass region was discovered where a Griffiths-like breakdown of long-range spin order occurs.

  8. Highly Efficient Domain Walls Injection in Perpendicular Magnetic Anisotropy Nanowire

    PubMed Central

    Zhang, S. F.; Gan, W. L.; Kwon, J.; Luo, F. L.; Lim, G. J.; Wang, J. B.; Lew, W. S.

    2016-01-01

    Electrical injection of magnetic domain walls in perpendicular magnetic anisotropy nanowire is crucial for data bit writing in domain wall-based magnetic memory and logic devices. Conventionally, the current pulse required to nucleate a domain wall is approximately ~1012 A/m2. Here, we demonstrate an energy efficient structure to inject domain walls. Under an applied electric potential, our proposed Π-shaped stripline generates a highly concentrated current distribution. This creates a highly localized magnetic field that quickly initiates the nucleation of a magnetic domain. The formation and motion of the resulting domain walls can then be electrically detected by means of Ta Hall bars across the nanowire. Our measurements show that the Π-shaped stripline can deterministically write a magnetic data bit in 15 ns even with a relatively low current density of 5.34 × 1011 A/m2. Micromagnetic simulations reveal the evolution of the domain nucleation – first, by the formation of a pair of magnetic bubbles, then followed by their rapid expansion into a single domain. Finally, we also demonstrate experimentally that our injection geometry can perform bit writing using only about 30% of the electrical energy as compared to a conventional injection line. PMID:27098108

  9. Highly Efficient Domain Walls Injection in Perpendicular Magnetic Anisotropy Nanowire.

    PubMed

    Zhang, S F; Gan, W L; Kwon, J; Luo, F L; Lim, G J; Wang, J B; Lew, W S

    2016-01-01

    Electrical injection of magnetic domain walls in perpendicular magnetic anisotropy nanowire is crucial for data bit writing in domain wall-based magnetic memory and logic devices. Conventionally, the current pulse required to nucleate a domain wall is approximately ~10(12) A/m(2). Here, we demonstrate an energy efficient structure to inject domain walls. Under an applied electric potential, our proposed Π-shaped stripline generates a highly concentrated current distribution. This creates a highly localized magnetic field that quickly initiates the nucleation of a magnetic domain. The formation and motion of the resulting domain walls can then be electrically detected by means of Ta Hall bars across the nanowire. Our measurements show that the Π-shaped stripline can deterministically write a magnetic data bit in 15 ns even with a relatively low current density of 5.34 × 10(11) A/m(2). Micromagnetic simulations reveal the evolution of the domain nucleation - first, by the formation of a pair of magnetic bubbles, then followed by their rapid expansion into a single domain. Finally, we also demonstrate experimentally that our injection geometry can perform bit writing using only about 30% of the electrical energy as compared to a conventional injection line. PMID:27098108

  10. Highly Efficient Domain Walls Injection in Perpendicular Magnetic Anisotropy Nanowire

    NASA Astrophysics Data System (ADS)

    Zhang, S. F.; Gan, W. L.; Kwon, J.; Luo, F. L.; Lim, G. J.; Wang, J. B.; Lew, W. S.

    2016-04-01

    Electrical injection of magnetic domain walls in perpendicular magnetic anisotropy nanowire is crucial for data bit writing in domain wall-based magnetic memory and logic devices. Conventionally, the current pulse required to nucleate a domain wall is approximately ~1012 A/m2. Here, we demonstrate an energy efficient structure to inject domain walls. Under an applied electric potential, our proposed Π-shaped stripline generates a highly concentrated current distribution. This creates a highly localized magnetic field that quickly initiates the nucleation of a magnetic domain. The formation and motion of the resulting domain walls can then be electrically detected by means of Ta Hall bars across the nanowire. Our measurements show that the Π-shaped stripline can deterministically write a magnetic data bit in 15 ns even with a relatively low current density of 5.34 × 1011 A/m2. Micromagnetic simulations reveal the evolution of the domain nucleation – first, by the formation of a pair of magnetic bubbles, then followed by their rapid expansion into a single domain. Finally, we also demonstrate experimentally that our injection geometry can perform bit writing using only about 30% of the electrical energy as compared to a conventional injection line.

  11. Magnetic Properties of Single Crystal Clinopyroxenes: Anisotropy of Remanence

    NASA Astrophysics Data System (ADS)

    Scott, G. R.; Feinberg, J. M.; Renne, P. R.

    2002-12-01

    (also by a factor of 4), reaching a minimum whenever the applied field is most perpendicular to the X and Z arrays. The saturation magnetization (Ms) is less variable, but shows 30% variations when the applied field is perpendicular to the X and Z arrays. Microscopic coercivity has been measured using the detailed hysteresis method of FORC analysis (First Order Reversal Curves). Each array of magnetites can be measured separately by applying the field perpendicular to the other array. Differences in the microcoercivity can be determined for each array, e.g. X=75-100mT while Z=85-125mT. Extreme anisotropy can be seen whenever the applied field is perpendicular to the plane of the arrays (Y direction), such that no microcoercivity population can be detected (up to 700mT) in the Y direction. For IRM, the remanence also appears to be null in the Y direction. The current challenge is to overcome these extreme restrictions in remanence anisotropy, while utilizing the equally extreme remanence stability to decode paleomagnetic field directions and intensities.

  12. Anisotropy of the magnetic susceptibility of gallium

    USGS Publications Warehouse

    Pankey, T., Jr.

    1960-01-01

    The bulk magnetic susceptibilities of single gallium crystals and polycrystalline gallium spheres were measured at 25??C. The following anisotropic diamagnetic susceptibilities were found: a axis (-0.119??0. 001)??10-6 emu/g, b axis (-0.416??0.002)??10 -6 emu/g, and c axis (-0.229??0.001) emu/g. The susceptibility of the polycrystalline spheres, assumed to be the average value for the bulk susceptibility of gallium, was (-0.257??0.003)??10-6 emu/g at 25??C, and (-0.299??0.003)??10-6 emu/g at -196??C. The susceptibility of liquid gallium was (0.0031??0.001) ??10-6 emu/g at 30??C and 100??C. Rotational diagrams of the susceptibilities in the three orthogonal planes of the unit cell were not sinusoidal. The anisotropy in the single crystals was presumably caused by the partial overlap of Brillouin zone boundaries by the Fermi-energy surface. The large change in susceptibility associated with the change in state was attributed to the absence of effective mass influence in the liquid state. ?? 1960 The American Institute of Physics.

  13. Magnetic and structural anisotropies of Co2FeAl Heusler alloy epitaxial thin films

    NASA Astrophysics Data System (ADS)

    Gabor, M. S.; Petrisor, T., Jr.; Tiusan, C.; Hehn, M.; Petrisor, T.

    2011-10-01

    This paper shows the correlation between chemical order, lattice strains, and magnetic properties of Heusler Co2FeAl films epitaxially grown on MgO(001). A detailed magnetic characterization is performed using vector-field magnetometery combined with a numerical Stoner-Wohlfarth analysis. We demonstrate the presence of three types of in-plane anisotropies: one biaxial, as expected for the cubic symmetry, and two uniaxial. The three anisotropies show different behavior with the annealing temperature. The biaxial anisotropy shows a monotonic increase. The uniaxial anisotropy that is parallel to the hard biaxial axes (related to chemical homogeneity) decreases, while the anisotropy that is supposed to have a magnetostatic origin remains constant.

  14. Artificially modified magnetic anisotropy in interconnected nanowire networks

    NASA Astrophysics Data System (ADS)

    Araujo, Elsie; Encinas, Armando; Velázquez-Galván, Yenni; Martínez-Huerta, Juan Manuel; Hamoir, Gaël; Ferain, Etienne; Piraux, Luc

    2015-01-01

    Interconnected or crossed magnetic nanowire networks have been fabricated by electrodeposition into a polycarbonate template with crossed cylindrical nanopores oriented +/-30° with respect to the surface normal. Tailor-made nanoporous polymer membranes have been designed by performing a double energetic heavy ion irradiation with fixed incidence angles. The Ni and Ni/NiFe nanowire networks have been characterized by magnetometry as well as ferromagnetic resonance and compared with parallel nanowire arrays of the same diameter and density. The most interesting feature of these nanostructured materials is a significant reduction of the magnetic anisotropy when the external field is applied perpendicular and parallel to the plane of the sample. This effect is attributed to the relative orientation of the nanowire axes with the applied field. Moreover, the microwave transmission spectra of these nanowire networks display an asymmetric linewidth broadening, which may be interesting for the development of low-pass filters. Nanoporous templates made of well-defined nanochannel network constitute an interesting approach to fabricate materials with controlled anisotropy and microwave absorption properties that can be easily modified by adjusting the relative orientation of the nanochannels, pore sizes and material composition along the length of the nanowire.

  15. An enhancement behavior of coercivity near TC in ferromagnetic films with uniaxial magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Dho, Joonghoe

    2012-08-01

    The temperature dependence of coercivity was investigated in CrO2 and La0.7Sr0.3MnO3 films with and without uniaxial magnetic anisotropy. When the magnetic field was applied along the uniaxial magnetic anisotropy axis, the coercivities of the CrO2 and La0.7Sr0.3MnO3 films showed remarkable enhancement behaviors near ferromagnetic transition temperature (TC). In contrast, CrO2 and La0.7Sr0.3MnO3 films without uniaxial magnetic anisotropy did not exhibit such an enhancement behavior. The temperature dependence of coercivity HC(T) for an aligned Stoner-Wohlfarth ferromagnet was theoretically studied based on a modified model of previously reported ones by He [Phys. Rev. B 75, 184424 (2007)] and Grimsditch [Phys. Rev. Lett. 90, 257201 (2003)]. Experimentally observed enhancement of coercivity near TC could be explained by an effect of a distribution of the local ordering temperatures ρ(TB) for magnetic grains. The qualitative behavior of HC(T) was investigated for three different types of uniaxial anisotropies: (i) magnetocrystalline anisotropy, (ii) strain-induced anisotropy, and (iii) shape anisotropy.

  16. Three tetracoordinate Co(II) complexes [Co(biq)X2] (X = Cl, Br, I) with easy-plane magnetic anisotropy as field-induced single-molecule magnets.

    PubMed

    Smolko, L; Černák, J; Dušek, M; Miklovič, J; Titiš, J; Boča, R

    2015-10-28

    Three mononuclear complexes [Co(biq)X2] (biq = 2,2'-biquinoline; X = Cl, Br, I) were prepared by a solvothermal method and characterized by single-crystal X-ray diffraction. In all three complexes the Co(ii) atom is tetrahedrally coordinated by one biq ligand bonded in a chelate manner and two halogenido ligands. Hydrogen bonding interactions (C-HX) along with the π-π interactions contribute to the stability of the formed packing. Magnetic measurements as well as ab initio calculations revealed that the complexes possess a sizable easy-plane magnetic anisotropy (D > 0). They display a superparamagnetic behaviour in an applied external field that culminates between BDC = 0.2-0.3 T. Two relaxation processes are observed; the faster can be analysed in terms of the direct and Orbach processes yielding U/kB = 42.6 K and τ0 = 1.9 × 10(-10) s for X = Cl, U/kB = 39.6 K and τ0 = 1.2 × 10(-10) s for X = Br and U/kB = 57.0 K and τ0 = 3.2 × 10(-13) s for X = I at BDC = 0.2 T. PMID:26391615

  17. Colossal anisotropy of the magnetic properties of doped lithium nitrodometalates

    NASA Astrophysics Data System (ADS)

    Antropov, V. P.; Antonov, V. N.

    2014-09-01

    We present a first-principles investigation of the electronic structure and physical properties of doped lithium nitridometalates Li2(Li1-xMx)N (LiMN) with M = Cr, Mn, Fe, Co, and Ni. The diverse properties include the equilibrium magnetic moments, magneto-crystalline anisotropy, magneto-optical Kerr spectra, and x-ray magnetic circular dichroism. We explain the colossal magnetic anisotropy in LiFeN by its unique electronic structure which ultimately leads to a series of unusual physical properties. The most unique property is a complete suppression of relativistic effects and freezing of orbital moments for in-plane orientation of the magnetization. This leads to the colossal spatial anisotropy of many magnetic properties including energy, Kerr, and dichroism effects. LiFeN is identified as an ultimate single-ion anisotropy system where a nearly insulating state can be produced by a spin orbital coupling alone. A very nontrivial strongly fluctuating and sign changing character of the magnetic anisotropy with electronic 3d-atomic doping is predicted theoretically. A large and highly anisotropic Kerr effect due to the interband transitions between atomic-like Fe 3d bands is found for LiFeN. A giant anisotropy of the x-ray magnetic circular dichroism for the Fe K spectrum and a very weak one for the Fe L2,3 spectra in LiFeN are also predicted.

  18. Low-field susceptibility anisotropy of some biotite crystals

    NASA Astrophysics Data System (ADS)

    Zapletal, Karel

    1990-10-01

    The low-field magnetic susceptibility anisotropy (LMA) of weakly magnetic rocks is dominated by paramagnetic minerals among which micas, and mainly biotite, is important. For this reason, the LMA of biotite crystals was investigated in detail. Natural biotite crystals (from ten localities) having a wide range of iron concentration were also studied by other methods, including optical microscopy, X-ray microanalysis, Mössbauer spectroscopy and induced isothermal remanent magnetization. Ferromagnetic inclusions disturbing the magnetic properties of biotite were revealed in some crystals. The measured mean bulk susceptibility of pure crystals (four localities) ranges from 1.0 × 10 -3 to 1.8 × 10 -3 SI and agrees with the susceptibility calculated from the iron concentration (ranging from 12 to 20 wt.%) determined for each specimen. The susceptibility ellipsoid of pure biotite crystals is rotational about the minimum susceptibility direction parallel to the crystallographic c'-axis, and the anisotropy degree ranges from 1.34 to 1.36.

  19. Magnetism behaviours dominated by the interplay of magnetic anisotropy and exchange coupling in local Co discs.

    PubMed

    Yang, En-Cui; Liu, Zhong-Yi; Zhang, Lei; Yang, Na; Zhao, Xiao-Jun

    2016-05-10

    Disc-like Co core-derived (4,4)- and (3,6)-connected layers, {[Co7(C2H5OH)1.5(H2O)0.5(Hdatrz)2(μ3-OH)4(ip)5]·2.5H2O·C2H5OH}n () and [Co7(H2O)4(ade)2(μ3-OH)6(sip)2]n () (Hdatrz = 3,5-diamino-1,2,4-triazole, ade(-) = adeninate, ip(2-) = isophthalate and sip(3-) = 5-sulfoisophthalate) were solvothermally generated and structurally and magnetically characterized. The effect of magnetic anisotropy and exchange coupling from the local Co cores on the resulting magnetism properties are discussed. A crystallographically asymmetric Co core in exhibited an unusual single-molecule magnet (SMM)-like response under zero dc field resulting from strong anisotropy generated by two different types of Co(II) polyhedra and highly anisotropic exchange interactions. By contrast, a highly symmetric Co disc in belonging to the C2h point group showed only strong ferromagnetic exchange, to lead to an overall ST = 7/2 spin ground-state at low temperature. Thus, the interplay of magnetic anisotropy and exchange coupling has a great and complicated influence on the overall magnetic phenomena, which should be fully considered for the design and preparation of new Co(II)-SMMs. PMID:27089955

  20. Determination of anisotropy constants of protein encapsulated iron oxide nanoparticles by electron magnetic resonance

    NASA Astrophysics Data System (ADS)

    Li, Hongyan; Klem, Michael T.; Sebby, Karl B.; Singel, David J.; Young, Mark; Douglas, Trevor; Idzerda, Yves U.

    2009-02-01

    Angle-dependent electron magnetic resonance was performed on 4.9, 8.0, and 19 nm iron oxide nanoparticles encapsulated within protein capsids and suspended in water. Measurements were taken at liquid nitrogen temperature after cooling in a 1 T field to partially align the particles. The angle dependence of the shifts in the resonance field for the iron oxide nanoparticles (synthesized within Listeria-Dps, horse spleen ferritin, and cowpea chlorotic mottle virus) all show evidence of a uniaxial anisotropy. Using a Boltzmann distribution for the particles' easy-axis direction, we are able to use the resonance field shifts to extract a value for the anisotropy energy, showing that the anisotropy energy density increases with decreasing particle size. This suggests that surface anisotropy plays a significant role in magnetic nanoparticles of this size.

  1. Giant perpendicular magnetic anisotropy of an individual atom on two-dimensional transition metal dichalcogenides

    NASA Astrophysics Data System (ADS)

    Odkhuu, Dorj

    2016-08-01

    Exploring magnetism and magnetic anisotropy in otherwise nonmagnetic two-dimensional materials, such as graphene and transition metal dichalcogenides, is at the heart of spintronics research. Herein, using first-principles calculations we explore the possibility of reaching an atomic-scale perpendicular magnetic anisotropy by carefully exploring the large spin-orbit coupling, orbital magnetism, and ligand field in a suitable choice of a two-dimensional structure with transition metal adatoms. More specifically, we demonstrate perpendicular magnetic anisotropy energies up to an order of 100 meV per atom in individual ruthenium and osmium adatoms at a monosulfur vacancy in molybdenum disulfide. We further propose a phenomenological model where a spin state transition that involves hybridization between molybdenum a1 and adatomic e' orbitals is a possible mechanism for magnetization reversal from an in-plane to perpendicular orientation.

  2. Enhancement of perpendicular magnetic anisotropy thanks to Pt insertions in synthetic antiferromagnets

    NASA Astrophysics Data System (ADS)

    Bandiera, S.; Sousa, R. C.; Auffret, S.; Rodmacq, B.; Dieny, B.

    2012-08-01

    Synthetic antiferromagnets are of great interest as reference layers in magnetic tunnel junctions since they allow decreasing the dipolar coupling between the two magnetic electrodes and exhibit larger pinning fields than single reference layers. In this letter, we investigate the effect of the insertion of an ultrathin Pt layer in contact with the Ru spacer in synthetic antiferromagnets with perpendicular magnetic anisotropy. Surprisingly, for Ru thickness below 0.75 nm, the antiferromagnetic coupling amplitude through Ru first increases upon Pt insertion up to a critical Pt thickness (˜0.25 nm) above which coupling decreases. In addition, the corresponding increase of perpendicular magnetic anisotropy enhances the thermal stability of the structure.

  3. Magnetic anisotropy of the radula of chiton Acanthochiton rubrolinestus LISCHKE.

    PubMed

    Qian, Xia; Zhao, Jian-Gao; Liu, Chuan-Lin; Guo, Cheng-Hua

    2002-09-01

    The magnetic anisotropy of the whole radula, the major lateral radula teeth, and magnetic material in the major lateral radula teeth of the chiton Acanthochiton rubrolinestus LISCHKE have been studied by a magnetic torque meter and superconducting quantum interference device (SQUID) magnetometer. The length and width axes of the teeth are the easily magnetized axes, while the thickness axis is difficult to magnetize. The width and thickness axes of the radula are the easily magnetized axes, and the length axis is difficult to magnetize. The measurement results of the whole radula and the major lateral radula teeth agree well with each other. The magnetic anisotropy of the magnetic material is given as well as a possible distribution of the magnetic material in the major lateral radula teeth. PMID:12210567

  4. Anisotropic Magnetism in Field-Structured Composites

    SciTech Connect

    Anderson, Robert A.; Martin, James E.; Odinek, Judy; Venturini, Eugene

    1999-06-24

    Magnetic field-structured-composites (FSCs) are made by structuring magnetic particle suspensions in uniaxial or biaxial (e.g. rotating) magnetic fields, while polymerizing the suspending resin. A uniaxial field produces chain-like particle structures, and a biaxial field produces sheet-like particle structures. In either case, these anisotropic structures affect the measured magnetic hysteresis loops, with the magnetic remanence and susceptibility increased significantly along the axis of the structuring field, and decreased slightly orthogonal to the structuring field, relative to the unstructured particle composite. The coercivity is essentially unaffected by structuring. We present data for FSCs of magnetically soft particles, and demonstrate that the altered magnetism can be accounted for by considering the large local fields that occur in FSCs. FSCS of magnetically hard particles show unexpectedly large anisotropies in the remanence, and this is due to the local field effects in combination with the large crystalline anisotropy of this material.

  5. Pinned orbital moments – A new contribution to magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Audehm, P.; Schmidt, M.; Brück, S.; Tietze, T.; Gräfe, J.; Macke, S.; Schütz, G.; Goering, E.

    2016-05-01

    Reduced dimensionality and symmetry breaking at interfaces lead to unusual local magnetic configurations, such as glassy behavior, frustration or increased anisotropy. The interface between a ferromagnet and an antiferromagnet is such an example for enhanced symmetry breaking. Here we present detailed X-ray magnetic circular dichroism and X-ray resonant magnetic reflectometry investigations on the spectroscopic nature of uncompensated pinned magnetic moments in the antiferromagnetic layer of a typical exchange bias system. Unexpectedly, the pinned moments exhibit nearly pure orbital moment character. This strong orbital pinning mechanism has not been observed so far and is not discussed in literature regarding any theory for local magnetocrystalline anisotropy energies in magnetic systems. To verify this new phenomenon we investigated the effect at different temperatures. We provide a simple model discussing the observed pure orbital moments, based on rotatable spin magnetic moments and pinned orbital moments on the same atom. This unexpected observation leads to a concept for a new type of anisotropy energy.

  6. Induced Anisotropy in FeCo-Based Nanocrystalline Ferromagnetic Alloys (HITPERM) by Very High Field Annealing

    NASA Technical Reports Server (NTRS)

    Johnson, F.; Garmestani, H.; Chu, S.-Y.; McHenry, M. E.; Laughlin, D. E.

    2004-01-01

    Very high magnetic field annealing is shown to affect the magnetic anisotropy in FeCo-base nanocrystalline soft ferromagnetic alloys. Alloys of composition Fe(44.5)Co(44.5)Zr(7)B(4) were prepared by melt spinning into amorphous ribbons, then wound to form toroidal bobbin cores. One set of cores was crystallized in a zero field at 600 deg. C for 1 h, then, field annealed at 17 tesla (T) at 480 deg. C for 1 h. Another set was crystallized in a 17-T field at 480 deg. C for 1 h. Field orientation was transverse to the magnetic path of the toroidal cores. An induced anisotropy is indicated by a sheared hysteresis loop. Sensitive torque magnetometry measurements with a Si cantilever sensor indicated a strong, uniaxial, longitudinal easy axis in the zero-field-crystallized sample. The source is most likely magnetoelastic anisotropy, caused by the residual stress from nanocrystallization and the nonzero magnetostriction coefficient for this material. The magnetostrictive coefficient lambda(5) is measured to be 36 ppm by a strain gage technique. Field annealing reduces the magnitude of the induced anisotropy. Core loss measurements were made in the zero-field-crystallized, zero-field-crystallized- than-field-annealed, and field-crystallized states. Core loss is reduced 30%-50% (depending on frequency) by field annealing. X-ray diffraction reveals no evidence of crystalline texture or orientation that would cause the induced anisotropy. Diffusional pair ordering is thought to be the cause of the induced anisotropy. However, reannealing the samples in the absence of a magnetic field at 480 deg. C does not completely remove the induced anisotropy.

  7. Stress induced anisotropy in CoFeMn soft magnetic nanocomposites

    NASA Astrophysics Data System (ADS)

    Leary, A. M.; Keylin, V.; Ohodnicki, P. R.; McHenry, M. E.

    2015-05-01

    The use of processing techniques to create magnetic anisotropy in soft magnetic materials is a well-known method to control permeability and losses. In nanocomposite materials, field annealing below the Curie temperature results in uniaxial anisotropy energies up to ˜2 kJ/m3. Higher anisotropies up to ˜10 kJ/m3 result after annealing Fe-Si compositions under stress due to residual stress in the amorphous matrix acting on body centered cubic crystals. This work describes near zero magnetostriction Co80-x-yFexMnyNb4B14Si2 soft magnetic nanocomposites, where x and y < 8 at.% with close packed crystalline grains that show stress induced anisotropies up to ˜50 kJ/m3 and improved mechanical properties with respect to Fe-Si compositions. Difference patterns measured using transmission X-ray diffraction show evidence of affine strain with respect to the stress axis.

  8. Helicity, anisotropies, and their competition in a multiferroic magnet: Insight from the phase diagram

    NASA Astrophysics Data System (ADS)

    Gvozdikova, M. V.; Ziman, T.; Zhitomirsky, M. E.

    2016-07-01

    Motivated by the complex phase diagram of MnWO4, we investigate the competition between anisotropy, magnetic field, and helicity for the anisotropic next-nearest-neighbor Heisenberg model. Apart from two competing exchanges, which favor a spiral magnetic structure, the model features the biaxial single-ion anisotropy. The model is treated in the real-space mean-field approximation and the phase diagram containing various incommensurate and commensurate states is obtained for different field orientations. We discuss the similarities and differences of the theoretical phase diagram and the experimental diagram of MnWO4.

  9. Large E-field tunability of magnetic anisotropy and ferromagnetic resonance frequency of co-sputtered Fe50Co50-B film

    NASA Astrophysics Data System (ADS)

    Li, Shandong; Xue, Qian; Du, Honglei; Xu, Jie; Li, Qiang; Shi, Zhipeng; Gao, Xiaoyang; Liu, Ming; Nan, Tianxiang; Hu, Zhongqiang; Sun, Nian X.; Shao, Weiquan

    2015-05-01

    Fe27.45Co30.19B42.36 (referred to as FeCoB) films with 100 nm in thickness were co-sputtered on (011)-cut lead zinc niobate-lead titanate (PZN-PT) single crystal substrate under RF powers of 80 W for Fe50Co50 target and 120 W for B target, respectively. The anisotropy field HK of the FeCoB/PZN-PT multiferroic composite is increased by more than 10 times, from 56 to 663 Oe under the E-field from 0 to 7 kV/cm due to the strong magnetoelectric coupling, corresponding to a large tunability of HK of 86.7 Oe cm/kV. At the same time, the self-bias ferromagnetic resonance frequency fFMR is dramatically shifted upwards by an electric field from 2.57 to 9.02 GHz with an increment of 6.45 GHz, corresponding to E-field tunablity of fFMR 921.4 MHz.cm/kV. These features demonstrate that FeCoB/PZN-PT multiferroic laminates prepared under an integrated circuits process are promising in fabrication of E-field tunable monolithic microwave integrated circuits (MMIC) devices and their components.

  10. Ferromagnetism and strong magnetic anisotropy of the PbMnBO4 orthoborate single crystals

    NASA Astrophysics Data System (ADS)

    Pankrats, A.; Sablina, K.; Eremin, M.; Balaev, A.; Kolkov, M.; Tugarinov, V.; Bovina, A.

    2016-09-01

    The PbMnBO4 orthoborate single crystals were first grown and their magnetic properties and ferromagnetic resonance were studied. It was found that the ferromagnetic state below the Curie temperature TC=31 K is characterized by the strong magnetic anisotropy. The significant effective anisotropy fields of PbMnBO4 determine the energy gap in the FMR spectrum, which is extraordinary large for ferromagnets (112 GHz at T=4.2 K). It was shown that the static Jahn-Teller effect characteristic of the Mn3+ ion leads to both the ferromagnetic ordering and the strong magnetic anisotropy in the crystal. In the strong external magnetic field the induced ferromagnetic ordering is retained in the crystal above the Curie temperature up to the temperatures multiply higher than TC. A weak anomaly of the dielectric permittivity was observed in PbMnBO4 at the Curie temperature at which the long-range ferromagnetic order is established.

  11. Understanding the magnetic anisotropy in Fe-Si amorphous alloys

    SciTech Connect

    Diaz, J.; Hamdan, N.M.; Jalil, P.; Hussain, Z.; Valvidares, S.M.; Alameda, J.M.

    2002-08-01

    The origin of the magnetic anisotropy in a very disordered Fe-Si alloy has been investigated. The alloy containing 40 percent at. Si was prepared in the form of a thin film in a DC magnetron sputtering chamber. Structural disorder was obtained from Extended X-ray Absorption Fine Structure spectroscopy. The uniformity and lack of inhomogeneities at a microscopic level was checked by measuring their transverse magnetic susceptibility and hysteresis loops. The orbital component of the magnetic moment was measured by X-ray Magnetic Circular Dichroism spectroscopy. The orbital moment was extraordinary high, 0.4mB. Such a high value contrasted with the relatively small uniaxial anisotropy energy of the thin film (2kJ/m3). This suggests that the cause of the magnetic anisotropy in this alloy was a small degree of correlation in the orientation of the local orbital moments along a preferential direction.

  12. Anisotropy of electric resistance and upper critical field in magnetic superconductor Dy0.6Y0.4Rh3.85Ru0.15B4

    NASA Astrophysics Data System (ADS)

    Terekhov, A. V.; Zolochevskii, I. V.; Khristenko, E. V.; Ishchenko, L. A.; Bezuglyi, E. V.; Zaleski, A.; Khlybov, E. P.; Lachenkov, S. A.

    2016-05-01

    We have measured temperature dependencies of the electric resistance R and upper critical magnetic field Hc2 of a magnetic superconductor Dy0.6Y0.4Rh3.85Ru0.15B4. The measurements were made for different angles φ of the magnetic field inclination to the direction of measuring current and revealed strong anisotropy of the behavior of R(T) and the values of Hc2(T). By using the Werthamer-Gelfand-Hohenberg theory, we determined the Maki parameter α and the parameter of the spin-orbital interaction. For φ =0∘ and 90° both parameters are close to zero, thus the magnitude of Hc2(0) ≈ 38 kOe is basically limited by the orbital effect. At φ =45∘ , a large value of α = 4.2 indicates dominating role of the spin-paramagnetic effect in the suppression of Hc2(0) down to 8.8 kOe. We suggest that such behavior of R(T) and Hc2(T) is caused by internal magnetism of the Dy atoms which may strongly depend on the magnetic field orientation.

  13. Stabilization of Magnetic Antivortices and the role of Shape Anisotropy

    NASA Astrophysics Data System (ADS)

    Asmat-Uceda, Martin; Li, Lin; Shaw, Brian; Haldar, Arabinda; Buchanan, Kristen

    2014-03-01

    Magnetic vortices have attracted a great deal of interest in recent years due to their potential for applications such as data storage, microwave resonators, magnonic crystals, etc. Magnetic antivortices (AV) are expected to possess similarly interesting physical attributes; however, they have not been explored with the same intensity. The AV spin configuration may present some advantages over vortices, especially for channeling spin waves emitted from the dynamic core reversal and for de-coupling spin-transfer torque effects from parasitic Oersted fields. Currently only a few geometries have been identified that reliably promote the formation of an AV, thus limiting the study of their properties. We recently demonstrated a method to form AV's in pound-key-like structures made of Permalloy (Haldar et al. APL 102, 112401, 2013). Here we investigate the dependence of the reliability of the AV formation on the details of the geometry of these structures. Magneto-optical Kerr effect (MOKE) hysteresis and magnetic force microscopy measurements show that the coercive field is also the nucleation field for the AV's. Micromagnetic simulations agree well with the experiments and highlight the role of shape anisotropy in the AV formation.

  14. Structure of nanoparticles in transformer oil-based magnetic fluids, anisotropy of acoustic attenuation

    NASA Astrophysics Data System (ADS)

    Kúdelčík, Jozef; Bury, Peter; Kopčanský, Peter; Timko, Milan

    2015-08-01

    The anisotropy of acoustic attenuation in transformer oil-based magnetic fluids upon the external magnetic field was studied to discover the structure of nanoparticles. When a magnetic field is increased, the interaction between the external magnetic field and the magnetic moments of the nanoparticles leads to the aggregation of magnetic nanoparticles and following clusters formation. However, the temperature of magnetic fluids and the concentration of nanoparticles also have very important influence on the structural changes. The measurement of the dependence of the acoustic attenuation on the angle between the magnetic field direction and acoustic wave vector (anisotropy) can give the useful information about the structure of magnetic nanoparticles formations. In the present, the results of anisotropy measurements of the transformer oil-based magnetic fluids are described and using appropriate theory the basic parameters of clusters are calculated. On the basis of the performed calculations, the proportion of the acoustic wave energy used for excitation of the translational and rotational degrees of freedom was also established.

  15. Control of magnetic anisotropy in Pt/Co system using ionic liquid gating

    NASA Astrophysics Data System (ADS)

    Hirai, Takamasa; Koyama, Tomohiro; Obinata, Aya; Hibino, Yuki; Miwa, Kazumoto; Ono, Shimpei; Kohda, Makoto; Chiba, Daichi

    2016-06-01

    The magnetic anisotropy of the Pt/Co system under ionic liquid gating was studied. A comparison of results obtained using samples under the gating and those subjected to mild oxidization by oxygen plasma ashing suggested that the anodic oxidization of the Co layer could be one of the causes of the large modulation observed in the magnetic anisotropy. However, the charge accumulation effect was probably dominant when the Co layer was on the cathode side. The experiments presented here are expected to aid in elucidating the mechanism by which electric fields affect magnetism.

  16. Orienting Paramecium with intense static magnetic fields

    NASA Astrophysics Data System (ADS)

    Valles, James M., Jr.; Guevorkian, Karine; Quindel, Carl

    2004-03-01

    Recent experiments on cell division suggest the application of intense static magnetic fields as a novel tool for the manipulation of biological systems [1]. The magnetic field appears to couple to the intrinsic anisotropies in the diamagnetic components of the cells. Here, we present measurements of the intrinsic average diamagnetic anisotropy of the whole single celled ciliate, Paramecium Caudatum. Magnetic fields, 2.5 T < B < 8 T were applied to immobilized (non-swimming) Paramecium Caudatum that were suspended in a density matched medium. The organisms align with their long axis parallel to the applied magnetic field. Their intrinsic diamagnetic anisotropy is 3x10-11 in cgs units. We will discuss the implications of these results for employing magnetic fields to probe the behavior of swimming Paramecium. [1] J. M. Valles, Jr. et al., Expt. Cell Res.274, 112-118 (2002).

  17. Magnetic anisotropy and reversal mechanisms in dual layer exchanged coupled perpendicular media

    NASA Astrophysics Data System (ADS)

    Thomson, T.; Lengsfield, B.; Do, H.; Terris, B. D.

    2008-04-01

    We report the magnetic properties of perpendicular media with a layered structure in which a high anisotropy, segregated, granular CoCrPt-oxide base layer is capped by a lower anisotropy CoCrPt-based film. Anisotropy field (Hk) data show that for the thickness of oxide media studied here, the measured value of Hk remains constant as cap thickness increases. This provides strong evidence that the anisotropy of the composite grain is controlled by the hard oxide layer and is not a simple average of the anisotropy of the oxide and cap layers. The reversal mechanism is explored by determining the angle dependent switching as a function of cap thickness. In the absence of a cap layer, the media show a Stoner-Wohlfarth-like reversal which becomes more Kondorsky-like [1/cos(θ)] when a critical cap thickness is reach, which we interpret as indicating greater lateral exchange coupling.

  18. Giant magnetic anisotropy and quantum tunneling of the magnetization in Li2(Li1-xFex)N

    NASA Astrophysics Data System (ADS)

    Jesche, Anton; McCallum, R. William; Thimmaiah, Srinivasa; Jacobs, Jenee L.; Taufour, Valentin; Kreyssig, Andreas; Houk, Robert S.; Bud'Ko, Sergey L.; Canfield, Paul C.

    2014-03-01

    The magnetic anisotropy of 3 d transition metals is usually considered to be weak, mainly due to the widely known paradigm of orbital quenching. However, a rare interplay of crystal electric field effects and spin-orbit coupling causes a large orbital contribution to the magnetic moment of iron in Li2(Li1-xFex)N. This leads, not only to large magnetic moments of ~ 5 μB per iron atom but, also, to an enormous magnetic anisotropy field that extrapolates to more than 200 Tesla. Magnetic hysteresis emerges for T <= 50 K and the coercivity fields of more than 11 Tesla exceed even the hardest 4 f electron based ferromagnets. Li2(Li1-xFex)N not only has a clear and remarkable anisotropy, generally not associated with iron moments, but also shows time-dependence more consistent with molecular magnets. In particular for low iron concentrations x << 1 the spin-inversion is dominated by a macroscopic tunneling process rather than by thermal excitations. It is shown that the huge magnetic anisotropy makes Li2(Li1-xFex)N (i) an ideal model system to study macroscopic quantum effects at elevated temperatures and (ii) a basis for novel magnetic functional materials. This work is supported by the US DOE, Basic Energy Sciences under Contract No. DE-AC02-07CH11358.

  19. Structure organization and magnetic properties of microscale ferrogels: The effect of particle magnetic anisotropy.

    PubMed

    Ryzhkov, Aleksandr V; Melenev, Petr V; Balasoiu, Maria; Raikher, Yuriy L

    2016-08-21

    The equilibrium structure and magnetic properties of a ferrogel object of small size (microferrogel(MFG)) are investigated by coarse-grained molecular dynamics. As a generic model of a microferrogel (MFG), a sample with a lattice-like mesh is taken. The solid phase of the MFG consists of magnetic (e.g., ferrite) nanoparticles which are mechanically linked to the mesh making some part of its nodes. Unlike previous models, the finite uniaxial magnetic anisotropy of the particles, as it is the case for real ferrogels, is taken into account. For comparison, two types of MFGs are considered: MFG-1, which dwells in virtually non-aggregated state independently of the presence of an external magnetic field, and MFG-2, which displays aggregation yet under zero field. The structure states of the samples are analyzed with the aid of angle-resolved radial distribution functions and cluster counts. The results reveal the crucial role of the matrix elasticity on the structure organization as well as on magnetization of both MFGs. The particle anisotropy, which plays insignificant role in MFG-1 (moderate interparticle magnetodipole interaction), becomes an important factor in MFG-2 (strong interaction). There, the restrictions imposed on the particle angular freedom by the elastic matrix result in notable diminution of the particle chain lengths as well as the magnetization of the sample. The approach proposed enables one to investigate a large variety of MFGs, including those of capsule type and to purposefully choose the combination of their magnetoelastic parameters. PMID:27544124

  20. Dielectric and magnetic anisotropy of a nematic ytterbium complex

    SciTech Connect

    Dobrun, L. A. Sakhatskii, A. S.; Kovshik, A. P.; Ryumtsev, E. I.; Kolomiets, I. P.; Knyazev, A. A.; Galyametdinov, Yu. G.

    2015-05-15

    The sign and the magnitude of the dielectric anisotropy of an ytterbium-based paramagnetic nematic liquid crystal complex, namely, tris[1-(4-(4-propylcyclohexyl)phenyl)octane-1,3-dione]-[5,5'-di (heptadecile)-2,2'-bipyridine]ytterbium, are determined. The temperature dependence of the permittivity components of the complex is obtained in the temperature range of a nematic phase. The sign of the anisotropy of the magnetic susceptibility of this compound is experimentally determined.

  1. Thermal Stability of Magnetic States in Circular Thin-Film Nanomagnets with Large Perpendicular Magnetic Anisotropy

    NASA Astrophysics Data System (ADS)

    Chaves-O'Flynn, Gabriel

    The scaling of the energy barrier to magnetization reversal in thin-film nanomagnets with perpendicular magnetization as a function of their lateral size is of great interest and importance for high-density magnetic random access memory devices. Experimental studies of such elements show either a quadratic or linear dependence of the energy barrier on element diameter. I will discuss a theoretical model we developed to determine the micromagnetic configurations that set the energy barrier for thermally activated reversal of a thin disk with perpendicular magnetic anisotropy as a function of disk diameter. We find a critical length in the problem that is set by the exchange and effective perpendicular magnetic anisotropy energies, with the latter including the size dependence of the demagnetization energy. For diameters smaller than this critical length, the reversal occurs by nearly coherent magnetization rotation and the energy barrier scales with the square of the diameter normalized to the critical length (for fixed film thickness), while for larger diameters, the transition state has a domain wall, and the energy barrier depends linearly on the normalized diameter. Simple analytic expressions are derived for these two limiting cases and verified using full micromagnetic simulations with the string method. Further, the effect of an applied field is considered and shown to lead to a plateau in the energy barrier versus diameter dependence at large diameters. Based on these finding I discuss the prospects and material challenges in the scaling of magnetic memory devices based on thin films with strong perpendicular magnetic anisotropy. In collaboration with G. Wolf, J. Z. Sun and A. D. Kent. Supported by NSF-DMR-1309202 and in part by Spin Transfer Technologies Inc. and the Nanoelectronics Research Initiative through the Institute for Nanoelectronics Discovery and Exploration.

  2. Hot-electron transport and magnetic anisotropy in epitaxial spin valves

    NASA Astrophysics Data System (ADS)

    Heindl, E.; Vancea, J.; Woltersdorf, G.; Back, C. H.

    2007-09-01

    We report on ballistic electron magnetic microscopy studies at room temperature using an epitaxially grown Fe34Co66/Au/Fe34Co66 trilayer. Local hysteresis loops are obtained as a function of the in-plane magnetic field angle. In order to understand the underlying local magnetization behavior, the magnetic anisotropies were determined by ferromagnetic resonance. These results served as input for simulations of the hysteresis loops, which are compared to magneto-optic Kerr effect and ballistic electron magnetic microscopy data of the spin valve. In doing so, the relative magnetization configuration of the spin valve can be calculated as a function of the external magnetic field, and the magnetization behavior during the reversal can be explained. Since different magnetization configurations of the spin valve are available, epitaxial spin valves allow multimagnetocurrent values, when the magnetic field is applied along different directions.

  3. Exchange coupling in hybrid anisotropy magnetic multilayers quantified by vector magnetometry

    SciTech Connect

    Morrison, C. Miles, J. J.; Thomson, T.; Anh Nguyen, T. N.; Fang, Y.; Dumas, R. K.; Åkerman, J.

    2015-05-07

    Hybrid anisotropy thin film heterostructures, where layers with perpendicular and in-plane anisotropy are separated by a thin spacer, are novel materials for zero/low field spin torque oscillators and bit patterned media. Here, we report on magnetization reversal and exchange coupling in a archetypal Co/Pd (perpendicular)-NiFe (in-plane) hybrid anisotropy system studied using vector vibrating sample magnetometry. This technique allows us to quantify the magnetization reversal in each individual magnetic layer, and measure of the interlayer exchange as a function of non-magnetic spacer thickness. At large (>1 nm) spacer thicknesses Ruderman-Kittel-Kasuya-Yosida-like exchange dominates, with orange-peel coupling providing a significant contribution only for sub-nm spacer thickness.

  4. Exchange coupling in hybrid anisotropy magnetic multilayers quantified by vector magnetometry

    NASA Astrophysics Data System (ADS)

    Morrison, C.; Miles, J. J.; Anh Nguyen, T. N.; Fang, Y.; Dumas, R. K.; Åkerman, J.; Thomson, T.

    2015-05-01

    Hybrid anisotropy thin film heterostructures, where layers with perpendicular and in-plane anisotropy are separated by a thin spacer, are novel materials for zero/low field spin torque oscillators and bit patterned media. Here, we report on magnetization reversal and exchange coupling in a archetypal Co/Pd (perpendicular)-NiFe (in-plane) hybrid anisotropy system studied using vector vibrating sample magnetometry. This technique allows us to quantify the magnetization reversal in each individual magnetic layer, and measure of the interlayer exchange as a function of non-magnetic spacer thickness. At large (>1 nm) spacer thicknesses Ruderman-Kittel-Kasuya-Yosida-like exchange dominates, with orange-peel coupling providing a significant contribution only for sub-nm spacer thickness.

  5. Research Update: Magnetoionic control of magnetization and anisotropy in layered oxide/metal heterostructures

    NASA Astrophysics Data System (ADS)

    Duschek, K.; Pohl, D.; Fähler, S.; Nielsch, K.; Leistner, K.

    2016-03-01

    Electric field control of magnetization and anisotropy in layered structures with perpendicular magnetic anisotropy is expected to increase the versatility of spintronic devices. As a model system for reversible voltage induced changes of magnetism by magnetoionic effects, we present several oxide/metal heterostructures polarized in an electrolyte. Room temperature magnetization of Fe-O/Fe layers can be changed by 64% when applying only a few volts in 1M KOH. In a next step, the bottom interface of the in-plane magnetized Fe layer is functionalized by an L10 FePt(001) underlayer exhibiting perpendicular magnetic anisotropy. During subsequent electrocrystallization and electrooxidation, well defined epitaxial Fe3O4/Fe/FePt heterostructures evolve. The application of different voltages leads to a thickness change of the Fe layer sandwiched between Fe-O and FePt. At the point of transition between rigid magnet and exchange spring magnet regime for the Fe/FePt bilayer, this induces a large variation of magnetic anisotropy.

  6. Correlations, spin-charge separation, and magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Skomski, Ralph; Manchanda, Priyanka

    2015-03-01

    Much of the physics of condensed matter reflects electron-electron correlations. On an independent-electron level, correlations are described by a single Slater determinant with broken spin symmetry. This approach includes Hund's rule correlations as well the LSDA and LSDA+U approximations to density-functional theory (DFT). However, from Kondo and heavy-fermion systems it is known that the independent-electron approach fails to describe spin-charge separation in strongly correlated systems, necessitating the use of two or more Slater determinants. Using first-principle and model calculations, we show that spin-charge separation strongly affects the leading rare-earth anisotropy contribution in top-end permanent magnet materials such as Nd2Fe14B and SmCo5. Explicit correlation results are obtained for two limiting cases. First, we derive the density functional for tripositive rare-earth ions in a Bethe-type crystal field. The potential looks very different from the LSDA(+U) potentials, including gradient corrections. Second, we use a simple model to show that Kondo-type spin-charge separation yield a rare-earth anisotropy contribution absent in the independent-electron approach. This research is supported by DOE (DE-FG02-04ER46152).

  7. Magnetostriction of rare-earth random magnetic anisotropy spin glasses

    SciTech Connect

    del Moral, A.; Arnaudas, J.I.

    1989-05-01

    A model of magnetostriction for single-ion random magnetic anisotropy (RMA) spin glasses (SG) is developed, the calculation being based on the replica technique. An overall uniform strain is assumed and coupled to the local easy axis (or easy plane) by an adequate projection. The obtained bulk magnetostriction becomes proportional to the average quadrupolar moment, which depends upon the assumed ferromagnetic uniform exchange, J/sub 0/, and the RMA crystal field (CEF), D/sub 0/, strengths. Magnetostriction measurements parallel (lambda/sub X/) and perpendicular (lambda/sub perpendicular/) to the applied magnetic field (up to 7 T) have been performed between 4.2 and 150 K (much larger than the SG temperature, T/sub SG/) for the amorphous spin glasses R/sub 40/Y/sub 23/Cu/sub 37/ (R = Tb, Dy, Ho, and Er). Anisotropic magnetostriction is a forced effect, with no sign of saturation, and is quite large well above T/sub SG/. The developed model fits quantitatively and remarkably well the temperature variation of the anisotropic magnetostriction, lambda/sub t/ = lambda/sub X/-lambda/sub perpendicular/, in the case of Tb, Dy, and Ho alloys. The values obtained from the fit for D/sub 0/, respectively, are +3.0, +1.25, and +0.6 K. For Er, D/sub 0/ becomes -0.37 K. The signs of D/sub 0/ are in agreement with having local axial anisotropy for the Tb, Dy, and Ho compounds, and planar for the Er one, in good agreement with the signs of the ..cap alpha../sub J/ Stevens quadrupolar parameter.

  8. Magnetic tunnel junction sensor with Co/Pt perpendicular anisotropy ferromagnetic layer

    SciTech Connect

    Wei, H. X.; Qin, Q. H.; Wen, Z. C.; Han, Prof. X. F.; Zhang, Xiaoguang

    2009-01-01

    Linear magnetoresistance (MR) is an important attribute for magnetic sensor designs for space applications, three dimensional detection of the magnetic field, and high field measurements. Here we demonstrate that a large linear MR of up to 22% can be achieved in a magnetic tunnel junction that consists of two ferromagnetic layers, one with out of plane and one with in plane magnetic anisotropy. The tunnelling magnetoresistance (TMR) is measured with the electrical current perpendicular to the film plane. The magnetic configuration of the device is analyzed.

  9. Growth Induced Magnetic Anisotropy in Crystalline and Amorphous Thin Films

    SciTech Connect

    Hellman, Frances

    1998-10-03

    OAK B204 Growth Induced Magnetic Anisotropy in Crystalline and Amorphous Thin Films. The work in the past 6 months has involved three areas of magnetic thin films: (1) amorphous rare earth-transition metal alloys, (2) epitaxial Co-Pt and hTi-Pt alloy thin films, and (3) collaborative work on heat capacity measurements of magnetic thin films, including nanoparticles and CMR materials.

  10. Axial Magnetic Anisotropy from Two Systems Fe2B and Co2B with Planar Anisotropy

    NASA Astrophysics Data System (ADS)

    Taufour, Valentin; Lamichhane, Tej; Bud'Ko, Sergey L.; Jesche, Anton; Goldman, Alan I.; Dennis, Kevin W.; McCallum, R. William; Antropov, Vladimir; Canfield, Paul C.

    2015-03-01

    Growth of single crystals of (Fe1-xCox)2B (0 <= x <= 1) and detailed characterization of their magnetic properties will be presented. Despite the fact that both Fe2B and Co2B show a planar anisotropy at room temperature, we observe a uniaxial anisotropy at intermediate doping which makes (Fe,Co)2B a promising system for permanent magnet applications in a system without rare-earth element. Comparison with recent band structure calculations will be presented. The temperature dependence of the anisotropy measured on single crystals from 2 K to 1000 K shows some unusual variations with an increase of the magnetic anisotropy with increasing temperature at some specific substitution. This work is supported by the Critical Materials Institute, an Energy Innovation Hub funded by the US DOE and by the Office of Basic Energy Science, Division of Materials Science and Engineering. Ames Laboratory is operated for the US DOE by Iowa State University under Contract No. DE-AC02-07CH11358.

  11. Proton resonant firehose instability: Temperature anisotropy and fluctuating field constraints

    NASA Astrophysics Data System (ADS)

    Gary, S. Peter; Li, Hui; O'Rourke, Sean; Winske, Dan

    1998-07-01

    The electromagnetic proton firehose instability may grow in a plasma if the proton velocity distribution is approximately bi-Maxwellian and T∥p>T⊥p, where the directional subscripts denote directions relative to the background magnetic field. Linear Vlasov dispersion theory in a homogeneous electron-proton plasma implies an instability threshold condition at constant maximum growth rate 1-T⊥p/T∥p=Sp/β∥pαp over 1<β∥p<=10 where β∥p≡8πnpT∥p/B02 and B0 is the background magnetic field. Here Sp and αp are fitting parameters and αp~=0.7. One- and two-dimensional initial value hybrid simulations of this growing mode are carried out under proton cyclotron resonant conditions in a homogeneous plasma on the initial domain 2<~β∥p<=100. The two-dimensional simulations show that enhanced fluctuations from this instability impose a bound on the proton temperature anisotropy of the form of the above equation with the fluid theory result αp~=1.0. On this domain both one- and two-dimensional simulations yield a new form for the upper bound on the fluctuating field energy density from the proton resonant firehose instability |δB|2/B02=SB+αBln(β∥p) where SB and αB are empirical parameters which are functions of the initial growth rate. This logarithmic behavior is qualitatively different from a fluid theory prediction and, like the anisotropy bound, should be subject to observational verification in any sufficiently homogeneous plasma in which the proton velocity distribution is approximately bi-Maxwellian.

  12. Effect of in-plane uniaxial anisotropy on self-organized magnetic structures generated by the Dzyaloshinskii-Moriya interaction

    NASA Astrophysics Data System (ADS)

    Oh, S. W.; Kwon, H. Y.; Won, C.

    2013-03-01

    The influences of uniaxial in-plane anisotropy on the properties of ordered magnetic structures generated by the DM interaction were investigated by performing Monte-Carlo simulated annealing. The uniaxial anisotropy aligns the magnetic structure along a specific direction and helps to organize magnetic skyrmions to form either a horizontal or a vertical hexagonal structure, depending on the anisotropy strength. The uniaxial in-plane anisotropy not only enhances the ordering of the structure but also enriches the phases of the system, which include a rectangular lattice structure of skyrmions and 1D skyrmion arrays separated by stripe domains. We investigate the formation conditions of the anisotropy strength and the external field for various magnetic phases.

  13. Origin of easy magnetization switching in magnetic tunnel junctions with voltage-controlled interfacial anisotropy

    PubMed Central

    Pertsev, Nikolay A.

    2013-01-01

    Spin-polarized currents represent an efficient tool for manipulating ferromagnetic nanostructures but the critical current density necessary for the magnetization switching is usually too high for applications. Here we show theoretically that, in magnetic tunnel junctions having electric-field-dependent interfacial anisotropy, the critical density may reduce down to a very low level (~104 A cm−2) when the junction combines small conductance with the proximity of free layer to a size-driven spin reorientation transition. The theory explains easy magnetization switching recently discovered in CoFeB/MgO/CoFeB tunnel junctions, surprisingly showing that it happens when the spin-transfer torque is relatively small, and provides a recipe for the fabrication of magnetic tunnel junctions suitable for industrial memory applications. PMID:24067783

  14. Slow magnetic relaxation in mononuclear seven-coordinate cobalt(II) complexes with easy plane anisotropy.

    PubMed

    Chen, Lei; Chen, Shu-Yang; Sun, Yi-Chen; Guo, Yu-Mei; Yu, Lu; Chen, Xue-Tai; Wang, Zhenxing; Ouyang, Z W; Song, You; Xue, Zi-Ling

    2015-07-01

    Two mononuclear seven-coordinate cobalt(II) complexes [Co(L)3(NO3)2] (L = 4-tert-butylpyridine, 1; L = isoquinoline, 2) were prepared and structurally analyzed by single-crystal X-ray crystallography. The coordination spheres of 1 and 2 exhibit distorted pentagonal bipyramid geometry. Analysis of their direct-current magnetic data reveals the existence of easy plane anisotropy (D > 0) with a small transverse anisotropy (E), which was further confirmed by high-field electron paramagnetic resonance (HFEPR) spectroscopy. Field-induced slow magnetic relaxations were observed under the applied dc field in complexes 1 and 2 by alternating-current magnetic susceptibility measurements. Importantly, these complexes are new instances of mononuclear high-coordinate cobalt(II)-based single-molecule magnets. PMID:26027953

  15. Giant magnetic anisotropy and tunnelling of the magnetization in Li2(Li1-xFex)N

    SciTech Connect

    Jesche, A.; McCallum, R. W.; Thimmaiah, S.; Jacobs, J. L.; Taufour, V.; Kreyssig, A.; Houk, R. S.; Bud’ko, S. L.; Canfield, P. C.

    2014-02-25

    Large magnetic anisotropy and coercivity are key properties of functional magnetic materials and are generally associated with rare earth elements. Here we show an extreme, uniaxial magnetic anisotropy and the emergence of magnetic hysteresis in Li2(Li1-xFex)N. An extrapolated, magnetic anisotropy field of 220 T and a coercivity field of over 11 T at 2 K outperform all known hard ferromagnets and single-molecular magnets. Steps in the hysteresis loops and relaxation phenomena in striking similarity to single-molecular magnets are particularly pronounced for x<<1 and indicate the presence of nanoscale magnetic centres. Quantum tunnelling, in the form of temperature-independent relaxation and coercivity, deviation from Arrhenius behaviour and blocking of the relaxation, dominates the magnetic properties up to 10 K. The simple crystal structure, the availability of large single crystals and the ability to vary the Fe concentration make Li2(Li1-xFex)N an ideal model system to study macroscopic quantum effects at elevated temperatures and also a basis for novel functional magnetic materials.

  16. Giant magnetic anisotropy and tunnelling of the magnetization in Li2(Li1-xFex)N

    NASA Astrophysics Data System (ADS)

    Jesche, A.; McCallum, R. W.; Thimmaiah, S.; Jacobs, J. L.; Taufour, V.; Kreyssig, A.; Houk, R. S.; Bud'Ko, S. L.; Canfield, P. C.

    2014-02-01

    Large magnetic anisotropy and coercivity are key properties of functional magnetic materials and are generally associated with rare earth elements. Here we show an extreme, uniaxial magnetic anisotropy and the emergence of magnetic hysteresis in Li2(Li1-xFex)N. An extrapolated, magnetic anisotropy field of 220 T and a coercivity field of over 11 T at 2 K outperform all known hard ferromagnets and single-molecular magnets. Steps in the hysteresis loops and relaxation phenomena in striking similarity to single-molecular magnets are particularly pronounced for x≪1 and indicate the presence of nanoscale magnetic centres. Quantum tunnelling, in the form of temperature-independent relaxation and coercivity, deviation from Arrhenius behaviour and blocking of the relaxation, dominates the magnetic properties up to 10 K. The simple crystal structure, the availability of large single crystals and the ability to vary the Fe concentration make Li2(Li1-xFex)N an ideal model system to study macroscopic quantum effects at elevated temperatures and also a basis for novel functional magnetic materials.

  17. Magnetic anisotropy in strained manganite films and bicrystal junctions

    NASA Astrophysics Data System (ADS)

    Demidov, V. V.; Ovsyannikov, G. A.; Petrzhik, A. M.; Borisenko, I. V.; Shadrin, A. V.; Gunnarsson, R.

    2013-04-01

    Transport and magnetic properties of La0.67Sr0.33MnO3 (LSMO) manganite thin films and bicrystal junctions were investigated. Epitaxial manganite films were grown on SrTiO3, LaAlO3, NdGaO3 (NGO), and (LaAlO3)0.3 + (Sr2AlTaO6)0.7 substrates, and their magnetic anisotropy were determined by two independent techniques of magnetic resonance spectroscopy. It was demonstrated that by using these techniques, a small (0.3%) anisotropy of crystal structure at the (110) surface plane of the orthorhombic NGO substrate leads to uniaxial magnetic anisotropy of the films in the plane of the substrate at least at the room temperature. It was found that on vicinal NGO substrates, the value of magnetic anisotropy strength can be varied in the range 100-200 Oe at T = 295 K by changing the substrate vicinal angle from 0° to 25°. Measurement of the magnetic anisotropy of manganite bicrystal junction demonstrated the presence of two ferromagnetic spin subsystems for both types of bicrystal boundaries with tilting of basal plane of manganite tilted bicrystal (TB-junction) and with rotation of crystallographic axes (RB-junction) used for comparison. The magnetoresistance of TB-junctions increases with decreasing temperature and the misorientation angle. Variation of bicrystal misorientation angle does not lead to change of misorientation of easy magnetic axes in the film parts forming TB-junction. Analysis of the voltage dependencies of bicrystal junction conductivity show that the low value of the magnetoresistance for the LSMO bicrystal junctions can be caused by two scattering mechanisms. The first one is the spin-flip of spin-polarized carriers due to the strong electron-electron interactions in a disordered layer at the bicrystal boundary at low temperatures and the second one is spin-flip by antiferromagnetic magnons at high temperatures.

  18. Perpendicular magnetic anisotropy and magnetization dynamics in oxidized CoFeAl films.

    PubMed

    Wu, Di; Zhang, Zhe; Li, Le; Zhang, Zongzhi; Zhao, H B; Wang, J; Ma, B; Jin, Q Y

    2015-01-01

    Half-metallic Co-based full-Heusler alloys with perpendicular magnetic anisotropy (PMA), such as Co2FeAl in contact with MgO, are receiving increased attention recently due to its full spin polarization for high density memory applications. However, the PMA induced by MgO interface can only be realized for very thin magnetic layers (usually below 1.3 nm), which would have strong adverse effects on the material properties of spin polarization, Gilbert damping parameter, and magnetic stability. In order to solve this issue, we fabricated oxidized Co50Fe25Al25 (CFAO) films with proper thicknesses without employing the MgO layer. The samples show controllable PMA by tuning the oxygen pressure (PO2) and CFAO thickness (tCFAO), large perpendicular anisotropy field of ~8.0 kOe can be achieved at PO2 = 12% for the sample of tCFAO = 2.1 nm or at PO2 = 7% for tCFAO = 2.8 nm. The loss of PMA at thick tCFAO or high PO2 results mainly from the formation of large amount of CoFe oxides, which are superparamagnetic at room temperature but become hard magnetic at low temperatures. The magnetic CFAO films, with strong PMA in a relatively wide thickness range and small intrinsic damping parameter below 0.028, would find great applications in developing advanced spintronic devices. PMID:26190066

  19. Resolving the controversy of a possible relationship between perpendicular magnetic anisotropy and the magnetic damping parameter

    SciTech Connect

    Shaw, Justin M.; Nembach, Hans T.; Silva, T. J.

    2014-08-11

    We use broadband ferromagnetic resonance spectroscopy to systematically measure the Landau-Lifshitz damping parameter, perpendicular anisotropy, and the orbital moment asymmetry in Co{sub 90}Fe{sub 10}/Ni multilayers. No relationship is found between perpendicular magnetic anisotropy and the damping parameter in this material. However, inadequate accounting for inhomogeneous linewidth broadening, spin-pumping, and two-magnon scattering could give rise to an apparent relationship between anisotropy and damping. In contrast, the orbital-moment asymmetry and the perpendicular anisotropy are linearly proportional to each other. These results demonstrate a fundamental mechanism by which perpendicular anisotropy can be varied independently of the damping parameter.

  20. Role of the substrate on the magnetic anisotropy of magnetite thin films grown by ion-assisted deposition

    NASA Astrophysics Data System (ADS)

    Prieto, Pilar; Prieto, José Emilio; Gargallo-Caballero, Raquel; Marco, José Francisco; de la Figuera, Juan

    2015-12-01

    Magnetite (Fe3O4) thin films were deposited on MgO (0 0 1), SrTiO3 (0 0 1), LaAlO3 (0 0 1) single crystal substrates as well on as silicon and amorphous glass in order to study the effect of the substrate on their magnetic properties, mainly the magnetic anisotropy. We have performed a structural, morphological and compositional characterization by X-ray diffraction, atomic force microscopy and Rutherford backscattering ion channeling in oxygen resonance mode. The magnetic anisotropy has been investigated by vectorial magneto-optical Kerr effect. The results indicate that the magnetic anisotropy is especially influenced by the substrate-induced microstructure. In-plane isotropy and uniaxial anisotropy behavior have been observed on silicon and glass substrates, respectively. The transition between both behaviors depends on grain size. For LaAlO3 substrates, in which the lattice mismatch between the Fe3O4 films and the substrate is significant, a weak in-plane fourfold magnetic anisotropy is induced. However when magnetite is deposited on MgO (0 0 1) and SrTiO3 (0 0 1) substrates, a well-defined fourfold in-plane magnetic anisotropy is observed with easy axes along [1 0 0] and [0 1 0] directions. The magnetic properties on these two latter substrates are similar in terms of magnetic anisotropy and coercive fields.

  1. Magnetization reversal mechanism of Nd-Fe-B films with perpendicular magnetic anisotropy

    SciTech Connect

    Liu Xiaoxi; Ishida, Go; Morisako, Akimitsu

    2011-04-01

    The microstructure and magnetic properties of Nd-Fe-B films with thicknesses from 100 nm to 3 nm have been investigated. All the films show excellent perpendicular magnetic anisotropy with a squareness ratio of 1 in the perpendicular direction and almost zero coercivity in the in-plane direction. Of particular interest is that the initial magnetization curves sensitively depended on the film thickness. Films thicker than 15 nm show steep initial magnetization curve. Although the films have coercivities larger than 21 kOe, the films can be fully magnetized from the thermally demagnetized state with a field as small as 5 kOe. With the decrease of film thickness to 5 nm, the initial magnetization curve becomes flat. The evolution of initial magnetization curves with film thickness can be understood by the microstructure of the films. Films with thickness of 15 nm show close-packed grains without any intergranular phases. Such microstructures lead to steep initial magnetization curves. On the other hand, when the film thickness decreased to 3 nm, the film thickness became nonuniform. Such microstructure leads to flat initial magnetization curves.

  2. Magnetic field induced anisotropy of 139La spin-lattice relaxation rates in stripe ordered La1.875Ba0.125CuO4

    NASA Astrophysics Data System (ADS)

    Baek, S.-H.; Utz, Y.; Hücker, M.; Gu, G. D.; Büchner, B.; Grafe, H.-J.

    2015-10-01

    We report 139La nuclear magnetic resonance studies performed on a La1.875Ba0.125CuO4 single crystal. The data show that the structural phase transitions (high-temperature tetragonal→low-temperature orthorhombic→low-temperature tetragonal phase) are of the displacive type in this material. The 139La spin-lattice relaxation rate T1-1 sharply upturns at the charge-ordering temperature TCO=54 K, indicating that charge order triggers the slowing down of spin fluctuations. Detailed temperature and field dependencies of the T1-1 below the spin-ordering temperature TSO=40 K reveal the development of enhanced spin fluctuations in the spin-ordered state for H ∥[001 ] , which are completely suppressed for large fields along the CuO2 planes. Our results shed light on the unusual spin fluctuations in the charge and spin stripe ordered lanthanum cuprates.

  3. Magnetic field induced anisotropy of 139La spin-lattice relaxation rates in stripe ordered La1.875Ba0.125CuO4

    DOE PAGESBeta

    S. -H. Baek; Gu, G. D.; Utz, Y.; Hucker, M.; Buchner, B.; Grafe, H. -J.

    2015-10-26

    We report 139La nuclear magnetic resonance studies performed on a La1.875Ba0.125CuO4 single crystal. The data show that the structural phase transitions (high-temperature tetragonal → low-temperature orthorhombic → low-temperature tetragonal phase) are of the displacive type in this material. The 139La spin-lattice relaxation rate T–11 sharply upturns at the charge-ordering temperature TCO = 54 K, indicating that charge order triggers the slowing down of spin fluctuations. Detailed temperature and field dependencies of the T–11 below the spin-ordering temperature TSO=40 K reveal the development of enhanced spin fluctuations in the spin-ordered state for H ∥ [001], which are completely suppressed for largemore » fields along the CuO2 planes. Lastly, our results shed light on the unusual spin fluctuations in the charge and spin stripe ordered lanthanum cuprates.« less

  4. Probing of the pairing state of HTSCs utilizing a-b plane magnetization anisotropy (abstract)

    NASA Astrophysics Data System (ADS)

    Buan, J.; Israeloff, N. E.; Huang, C. C.; Goldman, A. M.; Liu, J. Z.; Shelton, R. N.

    1994-05-01

    We have performed measurements of the a-b plane longitudinal and transverse magnetization anisotropy on an untwinned, high quality single crystal of LuBa2Cu3O7-x in magnetic fields below Hc1 as a function of temperature, from 2 K to the transition temperature and the angle between the field and a fixed direction in the a-b plane. When the superconducting order parameter has nodes on the Fermi surface, such as the case of the spin-singlet dx2-y2 order parameter, nonlinear effects associated with low-energy quasiparticles should become important.1 It was pointed out by Yip and Sauls that these effects will be most important at low temperatures. They should be observable in a measurement of the anisotropy of the magnetization or the magnetic torque. The magnetization is predicted to develop an anisotropic component transverse to the applied field. Anisotropic transverse magnetization with dx2-y2 symmetry is not seen in the temperature regime 5 to 25 K. Our results set stringent limits on the anisotropy of the transverse magnetization in this range. Within the resolution of our experiment no evidence for d-wave pairing is observed.

  5. The relation between ion temperature anisotropy and formation of slow shocks in collisionless magnetic reconnection

    NASA Astrophysics Data System (ADS)

    Higashimori, K.; Hoshino, M.

    2012-01-01

    We perform a two-dimensional simulation by using an electromagnetic hybrid code to study the formation of slow-mode shocks in collisionless magnetic reconnection in low beta plasmas, and we focus on the relation between the formation of slow shocks and the ion temperature anisotropy enhanced at the shock downstream region. It is known that as magnetic reconnection develops, the parallel temperature along the magnetic field becomes large in association with the anisotropic plasma sheet boundary layer ion beams, and this temperature anisotropy has a tendency to suppress the formation of slow shocks. On the basis of our simulation result, we found that the slow shock formation is suppressed due to the large temperature anisotropy near the X-type region, but the ion temperature anisotropy relaxes with increasing the distance from the magnetic neutral point. As a result, two pairs of current structures, which are the strong evidence of dissipation of magnetic field in slow shocks, are formed at the distance ∣x∣ ≥ 115 λi from the neutral point.

  6. Origin of Perpendicular Magnetic Anisotropy and Large Orbital Moment in Fe Atoms on MgO.

    PubMed

    Baumann, S; Donati, F; Stepanow, S; Rusponi, S; Paul, W; Gangopadhyay, S; Rau, I G; Pacchioni, G E; Gragnaniello, L; Pivetta, M; Dreiser, J; Piamonteze, C; Lutz, C P; Macfarlane, R M; Jones, B A; Gambardella, P; Heinrich, A J; Brune, H

    2015-12-01

    We report on the magnetic properties of individual Fe atoms deposited on MgO(100) thin films probed by x-ray magnetic circular dichroism and scanning tunneling spectroscopy. We show that the Fe atoms have strong perpendicular magnetic anisotropy with a zero-field splitting of 14.0±0.3  meV/atom. This is a factor of 10 larger than the interface anisotropy of epitaxial Fe layers on MgO and the largest value reported for Fe atoms adsorbed on surfaces. The interplay between the ligand field at the O adsorption sites and spin-orbit coupling is analyzed by density functional theory and multiplet calculations, providing a comprehensive model of the magnetic properties of Fe atoms in a low-symmetry bonding environment. PMID:26684139

  7. Pinned orbital moments - A new contribution to magnetic anisotropy.

    PubMed

    Audehm, P; Schmidt, M; Brück, S; Tietze, T; Gräfe, J; Macke, S; Schütz, G; Goering, E

    2016-01-01

    Reduced dimensionality and symmetry breaking at interfaces lead to unusual local magnetic configurations, such as glassy behavior, frustration or increased anisotropy. The interface between a ferromagnet and an antiferromagnet is such an example for enhanced symmetry breaking. Here we present detailed X-ray magnetic circular dichroism and X-ray resonant magnetic reflectometry investigations on the spectroscopic nature of uncompensated pinned magnetic moments in the antiferromagnetic layer of a typical exchange bias system. Unexpectedly, the pinned moments exhibit nearly pure orbital moment character. This strong orbital pinning mechanism has not been observed so far and is not discussed in literature regarding any theory for local magnetocrystalline anisotropy energies in magnetic systems. To verify this new phenomenon we investigated the effect at different temperatures. We provide a simple model discussing the observed pure orbital moments, based on rotatable spin magnetic moments and pinned orbital moments on the same atom. This unexpected observation leads to a concept for a new type of anisotropy energy. PMID:27151436

  8. Pinned orbital moments – A new contribution to magnetic anisotropy

    PubMed Central

    Audehm, P.; Schmidt, M.; Brück, S.; Tietze, T.; Gräfe, J.; Macke, S.; Schütz, G.; Goering, E.

    2016-01-01

    Reduced dimensionality and symmetry breaking at interfaces lead to unusual local magnetic configurations, such as glassy behavior, frustration or increased anisotropy. The interface between a ferromagnet and an antiferromagnet is such an example for enhanced symmetry breaking. Here we present detailed X-ray magnetic circular dichroism and X-ray resonant magnetic reflectometry investigations on the spectroscopic nature of uncompensated pinned magnetic moments in the antiferromagnetic layer of a typical exchange bias system. Unexpectedly, the pinned moments exhibit nearly pure orbital moment character. This strong orbital pinning mechanism has not been observed so far and is not discussed in literature regarding any theory for local magnetocrystalline anisotropy energies in magnetic systems. To verify this new phenomenon we investigated the effect at different temperatures. We provide a simple model discussing the observed pure orbital moments, based on rotatable spin magnetic moments and pinned orbital moments on the same atom. This unexpected observation leads to a concept for a new type of anisotropy energy. PMID:27151436

  9. Pattern-induced magnetic anisotropy in FePt thin films by ion irradiation

    SciTech Connect

    Jaafar, M.; Sanz, R.; McCord, J.; Jensen, J.; Schaefer, R.; Vazquez, M.; Asenjo, A.

    2011-03-01

    The magnetic properties of FePt thin films have been modified by exposing the samples to irradiation of 4 MeV Cl{sup 2+} ions. Patterned magnetic films, without modified topographical profile, were fabricated by irradiating the films through a shadowing micrometric mask. The structural changes, ascribed to the ion-beam-induced amorphization of the thin films, promote the modification of the magnetic anisotropy. In particular, the out-of-plane component of the magnetization decreases simultaneously with an enhancement of in-plane anisotropy by increasing ion fluence. Moreover, the nonirradiated regions present unexpected anisotropic behavior owing to the stray field of the irradiated regions. The control of this effect, which can have unwished consequences for the patterning of magnetic properties by ion bombardment, needs to be suitably addressed.

  10. Magnetic field sensor for isotropically sensing an incident magnetic field in a sensor plane

    NASA Technical Reports Server (NTRS)

    Pant, Bharat B. (Inventor); Wan, Hong (Inventor)

    2001-01-01

    A magnetic field sensor that isotropically senses an incident magnetic field. This is preferably accomplished by providing a magnetic field sensor device that has one or more circular shaped magnetoresistive sensor elements for sensing the incident magnetic field. The magnetoresistive material used is preferably isotropic, and may be a CMR material or some form of a GMR material. Because the sensor elements are circular in shape, shape anisotropy is eliminated. Thus, the resulting magnetic field sensor device provides an output that is relatively independent of the direction of the incident magnetic field in the sensor plane.

  11. Spin-orbit torque-assisted switching in magnetic insulator thin films with perpendicular magnetic anisotropy.

    PubMed

    Li, Peng; Liu, Tao; Chang, Houchen; Kalitsov, Alan; Zhang, Wei; Csaba, Gyorgy; Li, Wei; Richardson, Daniel; DeMann, August; Rimal, Gaurab; Dey, Himadri; Jiang, J S; Porod, Wolfgang; Field, Stuart B; Tang, Jinke; Marconi, Mario C; Hoffmann, Axel; Mryasov, Oleg; Wu, Mingzhong

    2016-01-01

    As an in-plane charge current flows in a heavy metal film with spin-orbit coupling, it produces a torque on and thereby switches the magnetization in a neighbouring ferromagnetic metal film. Such spin-orbit torque (SOT)-induced switching has been studied extensively in recent years and has shown higher efficiency than switching using conventional spin-transfer torque. Here we report the SOT-assisted switching in heavy metal/magnetic insulator systems. The experiments used a Pt/BaFe12O19 bilayer where the BaFe12O19 layer exhibits perpendicular magnetic anisotropy. As a charge current is passed through the Pt film, it produces a SOT that can control the up and down states of the remnant magnetization in the BaFe12O19 film when the film is magnetized by an in-plane magnetic field. It can reduce or increase the switching field of the BaFe12O19 film by as much as about 500 Oe when the film is switched with an out-of-plane field. PMID:27581060

  12. Control of magnetism by electric fields.

    PubMed

    Matsukura, Fumihiro; Tokura, Yoshinori; Ohno, Hideo

    2015-03-01

    The electrical manipulation of magnetism and magnetic properties has been achieved across a number of different material systems. For example, applying an electric field to a ferromagnetic material through an insulator alters its charge-carrier population. In the case of thin films of ferromagnetic semiconductors, this change in carrier density in turn affects the magnetic exchange interaction and magnetic anisotropy; in ferromagnetic metals, it instead changes the Fermi level position at the interface that governs the magnetic anisotropy of the metal. In multiferroics, an applied electric field couples with the magnetization through electrical polarization. This Review summarizes the experimental progress made in the electrical manipulation of magnetization in such materials, discusses our current understanding of the mechanisms, and finally presents the future prospects of the field. PMID:25740132

  13. Primordial statistical anisotropies: the effective field theory approach

    NASA Astrophysics Data System (ADS)

    Akbar Abolhasani, Ali; Akhshik, Mohammad; Emami, Razieh; Firouzjahi, Hassan

    2016-03-01

    In this work we present the effective field theory of primordial statistical anisotropies generated during anisotropic inflation involving a background U(1) gauge field. Besides the usual Goldstone boson associated with the breaking of time diffeomorphism we have two additional Goldstone bosons associated with the breaking of spatial diffeomorphisms. We further identify these two new Goldstone bosons with the expected two transverse degrees of the U(1) gauge field fluctuations. Upon defining the appropriate unitary gauge, we present the most general quadratic action which respects the remnant symmetry in the unitary gauge. The interactions between various Goldstone bosons leads to statistical anisotropy in curvature perturbation power spectrum. Calculating the general results for power spectrum anisotropy, we recover the previously known results in specific models of anisotropic inflation. In addition, we present novel results for statistical anisotropy in models with non-trivial sound speed for inflaton fluctuations. Also we identify the interaction which leads to birefringence-like effects in anisotropic power spectrum in which the speed of gauge field fluctuations depends on the direction of the mode propagation and the two polarization of gauge field fluctuations contribute differently in statistical anisotropy. As another interesting application, our EFT approach naturally captures interactions generating parity violating statistical anisotropies.

  14. Anisotropy of the magnetoviscous effect in ferrofluids containing nanoparticles exhibiting magnetic dipole interaction.

    PubMed

    Gerth-Noritzsch, M; Borin, D Yu; Odenbach, S

    2011-08-31

    The aim of this work has been the investigation of the anisotropy of the viscosity of a ferrofluid with magnetically interacting particles which are able to form structures in an applied magnetic field. The results of the experiments show a significant deviation from the case of a fluid without strong dipolar interactions. Furthermore, we have determined the dependence of the ratio of the viscosity coefficients on shear rate providing an insight into the microstructural reasons for the observed effects. PMID:21841240

  15. Size and voltage dependence of effective anisotropy in sub-100-nm perpendicular magnetic tunnel junctions

    NASA Astrophysics Data System (ADS)

    Piotrowski, Stephan K.; Bapna, Mukund; Oberdick, Samuel D.; Majetich, Sara A.; Li, Mingen; Chien, C. L.; Ahmed, Rizvi; Victora, R. H.

    2016-07-01

    Magnetic tunnel junctions with perpendicular magnetic anisotropy are investigated using a conductive atomic force microscope. The 1.23 -nm Co40Fe40B20 recording layer coercivity exhibits a size dependence which suggests single-domain behavior for diameters ≤100 nm. Focusing on devices with diameters smaller than 100 nm, we determine the effect of voltage and size on the effective device anisotropy Keff using two different techniques. Keff is extracted both from distributions of the switching fields of the recording and reference layers and from measurement of thermal fluctuations of the recording layer magnetization when a field close to the switching field is applied. The results from both sets of measurements reveal that Keff increases monotonically with decreasing junction diameter, consistent with the size dependence of the demagnetization energy density. We demonstrate that Keff can be controlled with a voltage down to the smallest size measured, 64 nm.

  16. Switching current density reduction in perpendicular magnetic anisotropy spin transfer torque magnetic tunneling junctions

    SciTech Connect

    You, Chun-Yeol

    2014-01-28

    We investigate the switching current density reduction of perpendicular magnetic anisotropy spin transfer torque magnetic tunneling junctions using micromagnetic simulations. We find that the switching current density can be reduced with elongated lateral shapes of the magnetic tunnel junctions, and additional reduction can be achieved by using a noncollinear polarizer layer. The reduction is closely related to the details of spin configurations during switching processes with the additional in-plane anisotropy.

  17. Magnetization reversal in magnetic dot arrays: Nearest-neighbor interactions and global configurational anisotropy

    NASA Astrophysics Data System (ADS)

    Van de Wiele, Ben; Fin, Samuele; Pancaldi, Matteo; Vavassori, Paolo; Sarella, Anandakumar; Bisero, Diego

    2016-05-01

    Various proposals for future magnetic memories, data processing devices, and sensors rely on a precise control of the magnetization ground state and magnetization reversal process in periodically patterned media. In finite dot arrays, such control is hampered by the magnetostatic interactions between the nanomagnets, leading to the non-uniform magnetization state distributions throughout the sample while reversing. In this paper, we evidence how during reversal typical geometric arrangements of dots in an identical magnetization state appear that originate in the dominance of either Global Configurational Anisotropy or Nearest-Neighbor Magnetostatic interactions, which depends on the fields at which the magnetization reversal sets in. Based on our findings, we propose design rules to obtain the uniform magnetization state distributions throughout the array, and also suggest future research directions to achieve non-uniform state distributions of interest, e.g., when aiming at guiding spin wave edge-modes through dot arrays. Our insights are based on the Magneto-Optical Kerr Effect and Magnetic Force Microscopy measurements as well as the extensive micromagnetic simulations.

  18. An algorithm to extract effective magnetic parameters of thin film with in-plane uniaxial magnetic anisotropy

    NASA Astrophysics Data System (ADS)

    Neo, C. P.; Ding, J.

    2010-05-01

    The calculation of high frequency complex permeability of thin ferromagnetic film requires the measured values of its saturation magnetization, anisotropic magnetic field intensity, resistivity, and thickness. It is often observed that the calculated permeability using the Landau-Lifshitz-Gilbert (LLG) theory does not agree well with the measured permeability of thin film with in-plane uniaxial magnetic anisotropy, owing to the measured anisotropic magnetic field intensity, saturation magnetization, etc., are not effective values at high frequency. In this work, the Landau-Lifshitz ferromagnetic resonance model is modified to take the skin depth effect into consideration. In the comparison study, its calculated magnetic permeability curves (real and imaginary) agrees very well with those calculated from the LLG model. In addition, an algorithm process to extract effective magnetic parameters (saturation magnetization Ms, magnetic anisotropy field Ha, and damping factor α) has been developed. The algorithm process has been tested for the reported magnetic permeability curves of two magnetic films (Si/NiFe/FeCoB and CoZrRe). The extracted parameters are well agreed with those reported. It is also reported that the consideration of skin depth effect is necessary for samples with lower electrical resistivity.

  19. Deciphering the origin of giant magnetic anisotropy and fast quantum tunnelling in Rhenium(IV) single-molecule magnets.

    PubMed

    Singh, Saurabh Kumar; Rajaraman, Gopalan

    2016-01-01

    Single-molecule magnets represent a promising route to achieve potential applications such as high-density information storage and spintronics devices. Among others, 4d/5d elements such as Re(IV) ion are found to exhibit very large magnetic anisotropy, and inclusion of this ion-aggregated clusters yields several attractive molecular magnets. Here, using ab intio calculations, we unravel the source of giant magnetic anisotropy associated with the Re(IV) ions by studying a series of mononuclear Re(IV) six coordinate complexes. The low-lying doublet states are found to be responsible for large magnetic anisotropy and the sign of the axial zero-field splitting parameter (D) can be categorically predicted based on the position of the ligand coordination. Large transverse anisotropy along with large hyperfine interactions opens up multiple relaxation channels leading to a fast quantum tunnelling of the magnetization (QTM) process. Enhancing the Re-ligand covalency is found to significantly quench the QTM process. PMID:26883278

  20. Deciphering the origin of giant magnetic anisotropy and fast quantum tunnelling in Rhenium(IV) single-molecule magnets

    PubMed Central

    Singh, Saurabh Kumar; Rajaraman, Gopalan

    2016-01-01

    Single-molecule magnets represent a promising route to achieve potential applications such as high-density information storage and spintronics devices. Among others, 4d/5d elements such as Re(IV) ion are found to exhibit very large magnetic anisotropy, and inclusion of this ion-aggregated clusters yields several attractive molecular magnets. Here, using ab intio calculations, we unravel the source of giant magnetic anisotropy associated with the Re(IV) ions by studying a series of mononuclear Re(IV) six coordinate complexes. The low-lying doublet states are found to be responsible for large magnetic anisotropy and the sign of the axial zero-field splitting parameter (D) can be categorically predicted based on the position of the ligand coordination. Large transverse anisotropy along with large hyperfine interactions opens up multiple relaxation channels leading to a fast quantum tunnelling of the magnetization (QTM) process. Enhancing the Re-ligand covalency is found to significantly quench the QTM process. PMID:26883278

  1. Deciphering the origin of giant magnetic anisotropy and fast quantum tunnelling in Rhenium(IV) single-molecule magnets

    NASA Astrophysics Data System (ADS)

    Singh, Saurabh Kumar; Rajaraman, Gopalan

    2016-02-01

    Single-molecule magnets represent a promising route to achieve potential applications such as high-density information storage and spintronics devices. Among others, 4d/5d elements such as Re(IV) ion are found to exhibit very large magnetic anisotropy, and inclusion of this ion-aggregated clusters yields several attractive molecular magnets. Here, using ab intio calculations, we unravel the source of giant magnetic anisotropy associated with the Re(IV) ions by studying a series of mononuclear Re(IV) six coordinate complexes. The low-lying doublet states are found to be responsible for large magnetic anisotropy and the sign of the axial zero-field splitting parameter (D) can be categorically predicted based on the position of the ligand coordination. Large transverse anisotropy along with large hyperfine interactions opens up multiple relaxation channels leading to a fast quantum tunnelling of the magnetization (QTM) process. Enhancing the Re-ligand covalency is found to significantly quench the QTM process.

  2. Effects of the magneto-crystalline anisotropy on the magnetic properties of Fe/Cr/Fe (110) trilayer

    NASA Astrophysics Data System (ADS)

    Bezerra, C. G.; Chesman, C.; Albuquerque, E. L.; Azevedo, A.

    2004-06-01

    In this paper we present a theoretical study about the influence of the magneto-crystalline anisotropy on the magnetic properties of magnetic metallic trilayers Fe/Cr/Fe (110). The theory is based on a realistic phenomenological model which includes the following contributions to the free magnetic energy: Zeeman, cubic and uniaxial anisotropy, as well as bilinear and biquadratic exchange energies. The experimental parameters used here are based on experimental data known from the literature. We present numerical results of magnetization versus external applied field to illustrate the behavior of the system. Our numerical results show that in some situations the saturation field can not be correctly determined by magnetoresistance measures.

  3. Hysteresis, critical fields and superferromagnetism of the film with perpendicular anisotropy

    NASA Astrophysics Data System (ADS)

    Kalita, V. M.; Kulyk, M. M.; Ryabchenko, S. M.

    2016-08-01

    This paper is focused on the analysis of hysteresis and critical phenomena of magnetization reversal of superferromagnetic (SFM) state in nanogranular (NG) Co/Al2O3 film with perpendicular anisotropy. It was demonstrated that the transition from the multidomain SFM state to the homogeneous SFM state, during the magnetization process, occurs critically. The value of the field of critical transition to the homogeneous state depends on the demagnetization field, granular anisotropy and interparticle exchange anisotropy. It turned out that the temperature dependence of the coercive force of the film, despite its SFM state, accords with the Neel-Brown formula for anisotropic single-domain ferromagnetic particles, but has an anomalous angular dependence. It was concluded that domain wall motion affects these features of the coercive field. The domain wall movement may occur due to the overturn of magnetic moments of particles in the boundaries between the superdomains. At the same time, the main factors influencing the coercivity are the anisotropy of the particles, which blocks their magnetic moment reorientation, and demagnetizing factor of the film. Together they lead to the anomalous angular dependence of the coercive field.

  4. Positive temperature coefficient of magnetic anisotropy in polyvinylidene fluoride (PVDF)-based magnetic composites

    PubMed Central

    Liu, Yiwei; Wang, Baomin; Zhan, Qingfeng; Tang, Zhenhua; Yang, Huali; Liu, Gang; Zuo, Zhenghu; Zhang, Xiaoshan; Xie, Yali; Zhu, Xiaojian; Chen, Bin; Wang, Junling; Li, Run-Wei

    2014-01-01

    The magnetic anisotropy is decreased with increasing temperature in normal magnetic materials, which is harmful to the thermal stability of magnetic devices. Here, we report the realization of positive temperature coefficient of magnetic anisotropy in a novel composite combining β-phase polyvinylidene fluoride (PVDF) with magnetostrictive materials (magnetostrictive film/PVDF bilayer structure). We ascribe the enhanced magnetic anisotropy of the magnetic film at elevated temperature to the strain-induced anisotropy resulting from the anisotropic thermal expansion of the β-phase PVDF. The simulation based on modified Stoner-Wohlfarth model and the ferromagnetic resonance measurements confirms our results. The positive temperature coefficient of magnetic anisotropy is estimated to be 1.1 × 102 J m−3 K−1. Preparing the composite at low temperature can enlarge the temperature range where it shows the positive temperature coefficient of magnetic anisotropy. The present results may help to design magnetic devices with improved thermal stability and enhanced performance. PMID:25311047

  5. Magnetic field sensor

    NASA Astrophysics Data System (ADS)

    Silva, Nicolas

    2012-09-01

    Earlier papers1-3 in this journal have described experiments on measuring the magnetic fields of current-carrying wires and permanent magnets using magnetic field probes of various kinds. This paper explains how to use an iPad and the free app MagnetMeter-3D Vector Magnetometer and Accelerometer4 (compass HD) to measure the magnetic fields.

  6. Enhancing the magnetic anisotropy of maghemite nanoparticles via the surface coordination of molecular complexes

    NASA Astrophysics Data System (ADS)

    Prado, Yoann; Daffé, Niéli; Michel, Aude; Georgelin, Thomas; Yaacoub, Nader; Grenèche, Jean-Marc; Choueikani, Fadi; Otero, Edwige; Ohresser, Philippe; Arrio, Marie-Anne; Cartier-Dit-Moulin, Christophe; Sainctavit, Philippe; Fleury, Benoit; Dupuis, Vincent; Lisnard, Laurent; Fresnais, Jérôme

    2015-12-01

    Superparamagnetic nanoparticles are promising objects for data storage or medical applications. In the smallest--and more attractive--systems, the properties are governed by the magnetic anisotropy. Here we report a molecule-based synthetic strategy to enhance this anisotropy in sub-10-nm nanoparticles. It consists of the fabrication of composite materials where anisotropic molecular complexes are coordinated to the surface of the nanoparticles. Reacting 5 nm γ-Fe2O3 nanoparticles with the [CoII(TPMA)Cl2] complex (TPMA: tris(2-pyridylmethyl)amine) leads to the desired composite materials and the characterization of the functionalized nanoparticles evidences the successful coordination--without nanoparticle aggregation and without complex dissociation--of the molecular complexes to the nanoparticles surface. Magnetic measurements indicate the significant enhancement of the anisotropy in the final objects. Indeed, the functionalized nanoparticles show a threefold increase of the blocking temperature and a coercive field increased by one order of magnitude.

  7. Magnetic anisotropy and high-spin effects in single-molecule transistors

    NASA Astrophysics Data System (ADS)

    Zyazin, Alexander; van den Berg, Johan; Osorio, Edgar; Konstantinidis, Nikos; Leijnse, Martin; May, Falk; Hofstetter, Walter; Danieli, Chiara; Cornia, Andrea; Wegewijs, Maarten; van der Zant, Herre

    2011-03-01

    Fabrication of single-molecule transistors where electron transport occurs through an individual molecule has become possible due to the recent progress in molecular electronics. Three-terminal configuration allows charging molecules and performing transport spectroscopy in multiple redox states. Single-molecule magnets combining large spin with uniaxial anisotropy are of special interest as appealing candidates for high density memory applications and quantum information processing. We study single-molecule magnets Fe 4 . Three-terminal junctions are fabricated using electromigration of gold nanowires followed by a self-breaking. High-spin Kondo effect and inelastic cotunneling excitations show up in transport measurements. Several excitations feature the energy close to the energy of zero-field splitting (ZFS) of a ground spin multiplet in bulk. This splitting is caused by the anisotropy and is a hallmark of single-molecule magnets. We observe nonlinear Zeeman effect due to a misalignment of an anisotropy axis and a magnetic field direction. The ZFS energy is increased in oxidized and reduced states of the molecule indicating enhancement of the anisotropy in these states.

  8. Temperature dependent magnetization in Co-base nanowire arrays: Role of crystalline anisotropy

    NASA Astrophysics Data System (ADS)

    Vivas, L. G.; Vázquez, M.; Vega, V.; García, J.; Rosa, W. O.; del Real, R. P.; Prida, V. M.

    2012-04-01

    Co, Co(1-x)Pdx, and Co(1-y)Niy nanowire arrays have been prepared by electrochemical template-assisted growth. Hcp, fcc or both phases are detected in Co nanowires depending on their length (300 nm to 40 μm) and on the content of Pd (0 ≤ x ≤ 0.4) and Ni (0 ≤ y ≤ 0.8). Their magnetic behavior has been studied under longitudinal and perpendicular applied fields. The effective magnetic anisotropy is mostly determined by the balance between the shape and the crystalline terms, the latter depending on the fractional volume of hcp phase with strong perpendicular anisotropy and fcc phase with weaker longitudinal anisotropy. The temperature dependence of remanence and coercivity and the eventual observation of compensation temperature is interpreted as due to the different temperature dependence of shape and hcp crystalline anisotropy. Optimum longitudinal magnetic anisotropy is achieved in low Pd-content CoPd nanowires and in short Co nanowires.

  9. Mapping of single-site magnetic anisotropy tensors in weakly coupled spin clusters by torque magnetometry.

    PubMed

    Rigamonti, Luca; Cornia, Andrea; Nava, Andrea; Perfetti, Mauro; Boulon, Marie-Emmanuelle; Barra, Anne-Laure; Zhong, Xiaoliang; Park, Kyungwha; Sessoli, Roberta

    2014-08-28

    Single-crystal torque magnetometry performed on weakly-coupled polynuclear systems provides access to a complete description of single-site anisotropy tensors. Variable-temperature, variable-field torque magnetometry was used to investigate triiron(III) complex [Fe3La(tea)2(dpm)6] (Fe3La), a lanthanum(III)-centred variant of tetrairon(III) single molecule magnets (Fe4) (H3tea = triethanolamine, Hdpm = dipivaloylmethane). Due to the presence of the diamagnetic lanthanoid, magnetic interactions among iron(III) ions (si = 5/2) are very weak (<0.1 cm(−1)) and the magnetic response of Fe3La is predominantly determined by single-site anisotropies. The local anisotropy tensors were found to have Di > 0 and to be quasi-axial with |Ei/Di| ~ 0.05. Their hard axes form an angle of approximately 70° with the threefold molecular axis, which therefore corresponds to an easy magnetic direction for the molecule. The resulting picture was supported by a High Frequency EPR investigation and by DFT calculations. Our study confirms that the array of peripheral iron(III) centres provides substantially noncollinear anisotropy contributions to the ground state of Fe4 complexes, which are of current interest in molecular magnetism and spintronics. PMID:25014192

  10. Thickness dependence of microwave magnetic properties in electrodeposited Fe-Co soft magnetic films with in-plane anisotropy

    NASA Astrophysics Data System (ADS)

    Yang, Xu; Wei, Jian-Qiang; Li, Xing-Hua; Gong, Lu-Qian; Wang, Tao; Li, Fa-Shen

    2012-02-01

    In this work, the thickness effect of Fe 52Co 48 soft magnetic films with in-plane anisotropy on static and microwave magnetic properties was investigated. The hysteresis loop results indicated that the static in-plane uniaxial anisotropy field increased from almost 0-60 Oe with increasing film thickness from 100 to 540 nm and well-defined in-plane uniaxial magnetic anisotropy can be obtained as the thickness reached 540 nm or larger. Based on Landau-Lifshitz-Gilbert (LLG) equation, the microwave complex permeability spectra were analyzed and well fitted. The LLG curve-fitting results indicated that the initial permeability increased from 106 to 142 and the resonant frequency was shifted from 4.95 to 4.29 GHz as the film thickness was varied from 540 to 1500 nm. Moreover, it was found that there was a discrepancy between the static and the dynamically determined anisotropy field, which can be explained by introducing an additional effective isotropic ripple field. The decreased ripple field was suggested to result in a significant decrease of damping coefficient from 0.109 to 0.038.