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Sample records for neutron induced prompt

  1. Prompt Fission Neutron Energy Spectra Induced by Fast Neutrons

    NASA Astrophysics Data System (ADS)

    Staples, Parrish Alan

    Prompt fission neutron energy spectra for ^{235}U and ^{239 }Pu have been measured for fission neutron energies greater than the energy of the incident neutrons inducing fission. The measurements were undertaken to investigate the shape dependence of the fission neutron spectra upon both the incident neutron energy and the mass of the nucleus undergoing fission. Measurements were made for both nuclides at the following incident neutron energies; 0.50 MeV, 1.50 MeV, 2.50 MeV and 3.50 MeV. The data are presented either as relative yields or as ratios of a measured spectrum to the ^{235}U spectrum at 0.50 MeV. Incident neutrons were produced by the ^7Li(p,n)^7Be reaction using a pulsed, bunched proton beam from the 5.5 MV Van de Graaff accelerator at the University of Massachusetts Lowell Pinanski Energy Center. The neutrons were detected by a thin liquid scintillator with good time resolution capabilities; time-of-flight techniques were used for neutron energy determination; in addition pulse-shape-discrimination was used to reduce gamma-ray background levels. The measurements are compared to calculations based on the Los Alamos Model of Madland and Nix to test its predictive capabilities. The data are fit by the Watt equation to determine the mean energy of the spectra, and to facilitate comparison of the results to previous measurements. The data are also compared directly to previous measurements.

  2. Prompt Emission in Fission Induced with Fast Neutrons

    NASA Astrophysics Data System (ADS)

    Wilson, J. N.; Lebois, M.; Halipré, P.; Oberstedt, S.; Oberstedt, A.

    Prompt gamma-ray and neutron emission data in fission integrates a large amount of information on the fission process and can shed light on the partition of energy. Measured emission spectra, average energies and multiplicities also provide important information for energy applications. While current reactors mostly use thermal neutron spectra, the future reactors of Generation IV will use fast neutron spectra for which little experimental prompt emission data exist. Initial investigations on prompt emission in fast neutron induced fission have recently been carried out at the LICORNE facility at the IPN Orsay, which exploits inverse reactions to produce naturally collimated, intense beams of neutrons. We report on first results with LICORNE to measure prompt fission gamma-ray spectra, average energies and multiplicities for 235U and 238U. Current improvements and upgrades being carried out on the LICORNE facility will also be described, including the development of a H2 gas target to reduce parasitic backgrounds and increase intensities, and the deployment of 11B beams to extend the effective LICORNE neutron energy range up to 12 MeV. Prospects for future experimental studies of prompt gamma-ray and neutron emission in fast neutron induced fission will be presented.

  3. Prompt fission neutron spectra in fast-neutron-induced fission of 238U

    NASA Astrophysics Data System (ADS)

    Desai, V. V.; Nayak, B. K.; Saxena, A.; Suryanarayana, S. V.; Capote, R.

    2015-07-01

    Prompt fission neutron spectrum (PFNS) measurements for the neutron-induced fission of 238U are carried out at incident neutron energies of 2.0, 2.5, and 3.0 MeV, respectively. The time-of-flight technique is employed to determine the energy of fission neutrons. The prompt fission neutron energy spectra so obtained are analyzed using Watt parametrization to derive the neutron multiplicity and average prompt fission neutron energy. The present experimental PFNS data are compared with the evaluated spectra taken from the ENDF/B-VII.1 library and the predictive calculations carried out using the empire-3.2 (Malta) code with built-in Los Alamos (LA) and Kornilov PFNS models. The sensitivity of the empire-3.2 LA model-calculated PFNS to the nuclear level density parameter of the average fission fragment and to the total kinetic energy is investigated. empire-3.2 LA model PFNS calculations that use Madland 2006-recommended values [D. G. Madland, Nucl. Phys. A 772, 113 (2006), 10.1016/j.nuclphysa.2006.03.013] of the total kinetic energy and the level density parameter a =A /(10 ±0.5 ) compare very well to measured data at all incident neutron incident energies.

  4. a Study of Prompt Neutron Emission in Thermal Neutron-Induced Fission of URANIUM-235.

    NASA Astrophysics Data System (ADS)

    Franklyn, Christopher Barry

    An original experiment was performed to measure the angular correlation of fission neutrons from thermal -neutron-induced fission of ('235)U, with respect to the light fission fragment direction, as a function of fragment mass division and neutron energy. A Monte Carlo model, with a realistic description of the fission fragment de -excitation process, was developed to simulate the observed neutron-fragment angular correlation data. The model was capable of investigating various possible forms of neutron emission which were classified into emission before, during and after full fragment acceleration, and correspondingly named scission acceleration and prompt neutron emission. Simulated neutron-fragment angular correlations displaying similar distributions with respect to the light fragment direction for different forms of neutron emission are shown to exhibit differing distributions when examined as a function of fragment mass division or neutron energy, thus illustrating the sensitivity of the experiment to the forms of neutron emission occurring in fission. A primary conclusion of the investigation was that neutron emission solely from fully accelerated fragments, whether isotropically or anisotropically emitted in the fragment centre of mass system, was unable to adequately describe the observed neutron-fragment angular correlations. Simulation of the fission process with some neutron emission before or during fragment acceleration exhibited a closer correspondence with observed phenomena. Within the scope of this work the form of neutron emission that produced the closest overall correspondence with experimental data was a simulation in which 20% of the emitted neutrons were isotropically emitted scission neutrons with a Maxwellian energy distribution of temperature 1.0 MeV. The remaining neutrons were emitted from fully accelerated fragments, being isotropic in the fragment centre of mass frame, except for the n-th(n > 1) neutrons from the light fragment, which

  5. Prompt Gamma Emission in Resonance Neutron Induced Fission of 239Pu

    NASA Astrophysics Data System (ADS)

    Ruskov, I.; Kopatch, Yu. N.; Panteleev, Ts.; Skoy, V. R.; Shvetsov, V. N.; Dermendjiev, E.; Janeva, N.; Pikelner, L. B.; Grigoriev, Yu. V.; Mezentseva, Zh. V.; Ivanov, I.

    The scientific interest in the resonance neutron induced capture and fission reactions on 239Pu is continuously rising during the last decade. From a practical point of view, this is because more precise data on capture and fission cross sections, fission fragment mass and kinetic energy distributions, variation of prompt fission neutron and gamma yields in the resonance neutron region, are needed for the modelling of new generation nuclear power plants and for nuclear spent fuel and waste transmutation. From a heuristic and fundamental point of view, such a research improves our knowledge and understanding of the fission phenomena itself. To achieve these goals more powerful neutron sources and more precise fission product detectors have to be used. At the Joint Institute for Nuclear Research (JINR) Frank Laboratory of Neutron Physics (FLNP), where already half a century the thermal and resonance neutron induced nuclear reactions are studied, a new electron accelerator driven white spectrum pulsed neutron source IREN has been built and successfully tested. The improved characteristics of this facility, in comparison with those of the former pulse neutron fast reactor IBR-30, will allow measuring some of the neutron-nuclear reaction data with better precision and accuracy. A new experimental setup for detecting gamma rays (and neutrons) has been designed and is under construction. It will consist of 2 rings (arrays) of 12 NaI(Tl) detectors each (or 1 array of 24 detectors) with variable ring diameter and distance between both rings. Such a setup will make possible not only to measure the multiplicity, energy and angular anisotropy of prompt fission gammas, but also to separate the contribution of prompt fission neutrons by their longer time-of-flight from the fissile target to the detectors. The signals from all the 24 detectors will be recorded simultaneously in digitized form and will be stored on the hard disk of the personal computer for further off

  6. Evaluating the 239Pu Prompt Fission Neutron Spectrum Induced by Thermal to 30 MeV Neutrons

    NASA Astrophysics Data System (ADS)

    Neudecker, D.; Talou, P.; Kawano, T.; Kahler, A. C.; Rising, M. E.; White, M. C.

    2016-03-01

    We present a new evaluation of the 239Pu prompt fission neutron spectrum (PFNS) induced by thermal to 30 MeV neutrons. Compared to the ENDF/B-VII.1 evaluation, this one includes recently published experimental data as well as an improved and extended model description to predict PFNS. For instance, the pre-equilibrium neutron emission component to the PFNS is considered and the incident energy dependence of model parameters is parametrized more realistically. Experimental and model parameter uncertainties and covariances are estimated in detail. Also, evaluated covariances are provided between all PFNS at different incident neutron energies. Selected evaluation results and first benchmark calculations using this evaluation are briefly discussed.

  7. Advanced Monte Carlo modeling of prompt fission neutrons for thermal and fast neutron-induced fission reactions on Pu239

    NASA Astrophysics Data System (ADS)

    Talou, P.; Becker, B.; Kawano, T.; Chadwick, M. B.; Danon, Y.

    2011-06-01

    Prompt fission neutrons following the thermal and 0.5 MeV neutron-induced fission reaction of Pu239 are calculated using a Monte Carlo approach to the evaporation of the excited fission fragments. Exclusive data such as the multiplicity distribution P(ν), the average multiplicity as a function of fragment mass ν¯(A), and many others are inferred in addition to the most used average prompt fission neutron spectrum χ(Ein,Eout), as well as average neutron multiplicity ν¯. Experimental information on these more exclusive data help constrain the Monte Carlo model parameters. The calculated average total neutron multiplicity is ν¯c=2.871 in very close agreement with the evaluated value ν¯e=2.8725 present in the ENDF/B-VII.0 library. The neutron multiplicity distribution P(ν) is in very good agreement with the evaluation by Holden and Zucker. The calculated average spectrum differs in shape from the ENDF/B-VII.0 spectrum, evaluated with the Madland-Nix model. In particular, we predict more neutrons in the low-energy tail of the spectrum (below about 300 keV) than the Madland-Nix calculations, casting some doubts on how much scission neutrons contribute to the shape of the low-energy tail of the spectrum. The spectrum high-energy tail is very sensitive to the total kinetic energy distribution of the fragments as well as to the total excitation energy sharing at scission. Present experimental uncertainties on measured spectra above 6 MeV are too large to distinguish between various theoretical hypotheses. Finally, comparisons of the Monte Carlo results with experimental data on ν¯(A) indicate that more neutrons are emitted from the light fragments than the heavy ones, in agreement with previous works.

  8. Material Classification by Analysis of Prompt Photon Spectra Induced by 14-Mev Neutrons

    NASA Astrophysics Data System (ADS)

    Barzilov, Alexander; Novikov, Ivan

    Neutron based technologies are widely used in the field of bulk material analysis. These methods employ characteristic prompt gamma rays induced by a neutron probe for classification of the interrogated object using the elemental parameters extracted from the spectral data. Automatic data analysis and material classification algorithms are required for applications where access to nuclear spectroscopy expertise is limited and/or the autonomous robotic operation is necessary. Data obtained with neutron based systems differ from elemental composition evaluations based on chemical formulae due to statistical nature of nuclear reactions, presence of shielding and cladding, and other environmental conditions. Experimental data that are produced by the spectral decomposition can be expressed graphically as sets of overlapping classes in a multidimensional space of measured elemental intensities. To discriminate between classes of various materials, decision-tree and pattern recognition algorithms were studied. Results of application of these methods to data sets obtained for a pulsed 14-MeV neutron generator based active interrogation system are discussed.

  9. Event-by-Event Fission Modeling of Prompt Neutrons and Photons from Neutron-Induced and Spontaneous Fission with FREYA

    NASA Astrophysics Data System (ADS)

    Vogt, Ramona; Randrup, Jorgen

    2013-04-01

    The event-by-event fission Monte Carlo code FREYA (Fission Reaction Event Yield Algorithm) generates large samples of complete fission events. Using FREYA, it is possible to obtain the fission products as well as the prompt neutrons and photons emitted during the fission process, all with complete kinematic information. We can therefore extract any desired correlation observables. Concentrating on ^239Pu(n,f), ^240Pu(sf) and ^252Cf(sf), we compare our FREYA results with available data on prompt neutron and photon emission and present predictions for novel fission observables that could be measured with modern detectors.

  10. Body composition to climate change studies - the many facets of neutron induced prompt gamma-ray analysis

    SciTech Connect

    Mitra,S.

    2008-11-17

    In-vivo body composition analysis of humans and animals and in-situ analysis of soil using fast neutron inelastic scattering and thermal neutron capture induced prompt-gamma rays have been described. By measuring carbon (C), nitrogen (N) and oxygen (O), protein, fat and water are determined. C determination in soil has become important for understanding below ground carbon sequestration process in the light of climate change studies. Various neutron sources ranging from radio isotopic to compact 14 MeV neutron generators employing the associated particle neutron time-of-flight technique or micro-second pulsing were implemented. Gamma spectroscopy using recently developed digital multi-channel analyzers has also been described.

  11. Comparative measurement of prompt fission γ -ray emission from fast-neutron-induced fission of 235U and 238U

    NASA Astrophysics Data System (ADS)

    Lebois, M.; Wilson, J. N.; Halipré, P.; Oberstedt, A.; Oberstedt, S.; Marini, P.; Schmitt, C.; Rose, S. J.; Siem, S.; Fallot, M.; Porta, A.; Zakari, A.-A.

    2015-09-01

    Prompt fission γ -ray (PFG) spectra have been measured in a recent experiment with the novel directional fast-neutron source LICORNE at the ALTO facility of the IPN Orsay. These first results from the facility involve the comparative measurement of prompt γ emission in fast-neutron-induced fission of 235U and 238U . Characteristics such as γ multiplicity and total and average radiation energy are determined in terms of ratios between the two systems. Additionally, the average photon energies were determined and compared with recent data on thermal-neutron-induced fission of 235U . PFG spectra are shown to be similar within the precision of the present measurement, suggesting that the extra incident energy does not significantly impact the energy released by prompt γ rays. The origins of some small differences, depending on either the incident energy or the target mass, are discussed. This study demonstrates the potential of the present approach, combining an innovative neutron source and new-generation detectors, for fundamental and applied research on fission in the near future.

  12. Evaluated Mean Values and Covariances for the Prompt Fission Neutron Spectrum of 239Pu induced by neutrons of 500 keV

    SciTech Connect

    Neudecker, Denise

    2014-07-10

    This document provides the numerical values of the evaluated prompt fission neutron spectrum for 239Pu induced by neutrons of 500 keV as well as relative uncertainties and correlations. This document also contains a short description how these data were obtained and shows plots comparing the evaluated results to experimental information as well as the corresponding ENDF/B-VII.1 evaluation.

  13. Prompt γ-rays from the Fast Neutron Induced Fission on 235,238U and 232Th

    NASA Astrophysics Data System (ADS)

    Lebois, M.; Wilson, J. N.; Halipré, P.; Leniau, B.; Matea, I.; Oberstedt, A.; Oberstedt, S.; Verney, D.

    Preliminary results from the first experiment using the LICORNE neutron source at the IPN Orsay are presented. Prompt fission gamma rays from fast-neutron induced fission of 238U, 232Th and 235U were detected. Thick samples of around 50 g of 238U and 232Th are used for the first part of the experiment. An ionisation chamber containing ∼ 10 mg samples of 238U and 235U to provide a fission trigger is used for the second part of the experiment. Gamma rays have been detected using 17 high efficiency BaF2 detectors and 6 LaBr3 scintillator detectors.

  14. Analysis of prompt fission neutrons in 235U(nth,f) and fission fragment distributions for the thermal neutron induced fission of 234U

    NASA Astrophysics Data System (ADS)

    Al-Adili, A.; Tarrío, D.; Hambsch, F.-J.; Göök, A.; Jansson, K.; Solders, A.; Rakopoulos, V.; Gustafsson, C.; Lantz, M.; Mattera, A.; Oberstedt, S.; Prokofiev, A. V.; Vidali, M.; Österlund, M.; Pomp, S.

    2016-06-01

    This paper presents the ongoing analysis of two fission experiments. Both projects are part of the collaboration between the nuclear reactions group at Uppsala and the JRC-IRMM. The first experiment deals with the prompt fission neutron multiplicity in the thermal neutron induced fission of 235U(n,f). The second, on the fission fragment properties in the thermal fission of 234U(n,f). The prompt fission neutron multiplicity has been measured at the JRC-IRMM using two liquid scintillators in coincidence with an ionization chamber. The first experimental campaign focused on 235U(nth,f) whereas a second experimental campaign is foreseen later for the same reaction at 5.5 MeV. The goal is to investigate how the so-called sawtooth shape changes as a function of fragment mass and excitation energy. Some harsh experimental conditions were experienced due to the large radiation background. The solution to this will be discussed along with preliminary results. In addition, the analysis of thermal neutron induced fission of 234U(n,f) will be discussed. Currently analysis of data is ongoing, originally taken at the ILL reactor. The experiment is of particular interest since no measurement exist of the mass and energy distributions for this system at thermal energies. One main problem encountered during analysis was the huge background of 235U(nth,f). Despite the negligible isotopic traces in the sample, the cross section difference is enormous. Solution to this parasitic background will be highlighted.

  15. Prompt fission neutron spectra of actinides

    DOE PAGESBeta

    Capote, R.; Chen, Y. -J.; Hambsch, F. -J.; Kornilov, N. V.; Lestone, J. P.; Litaize, O.; Morillon, B.; Neudecker, D.; Oberstedt, S.; Ohsawa, T.; et al

    2016-01-06

    Here, the energy spectrum of prompt neutrons emitted in fission (PFNS) plays a very important role in nuclear science and technology. A Coordinated Research Project (CRP) "Evaluation of Prompt Fission Neutron Spectra of Actinides" was established by the IAEA Nuclear Data Section in 2009, with the major goal to produce new PFNS evaluations with uncertainties for actinide nuclei.

  16. Neutron-induced fission: properties of prompt neutron and γ rays as a function of incident energy

    NASA Astrophysics Data System (ADS)

    Stetcu, I.; Talou, P.; Kawano, T.

    2016-06-01

    We have applied the Hauser-Feshbach statistical theory, in a Monte-Carlo implementation, to the de-excitation of fission fragments, obtaining a reasonable description of the characteristics of neutrons and gamma rays emitted before beta decays toward stability. Originally implemented for the spontaneous fission of 252Cf and the neutroninduced fission of 235U and 239Pu at thermal neutron energy, in this contribution we discuss the extension of the formalism to incident neutron energies up to 20 MeV. For the emission of pre-fission neutrons, at incident energies beyond second-chance fission, we take into account both the pre-equilibrium and statistical pre-fission components. Phenomenological parameterizations of mass, charge and TKE yields are used to obtain the initial conditions for the fission fragments that subsequently decay via neutron and emissions. We illustrate this approach for 239Pu(n,f).

  17. Energy Correlation of Prompt Fission Neutrons

    NASA Astrophysics Data System (ADS)

    Elter, Zs.; Pázsit, I.

    2016-03-01

    In all cases where neutron fluctuations in a branching process (such as in multiplicity measurements) are treated in an energy dependent description, the energy correlations of the branching itself (energy correlations of the fission neutrons) need to be known. To date, these are not known from experiments. Such correlations can be theoretically and numerically derived by modelling the details of the fission process. It was suggested earlier that the fact that the prompt neutrons are emitted from the moving fission targets, will influence their energy and angular distributions in the lab system, which possibly induces correlations. In this paper the influence of the neutron emission process from the moving targets on the energy correlations is investigated analytically and via numerical simulations. It is shown that the correlations are generated by the random energy and direction distributions of the fission fragments. Analytical formulas are derived for the two-point energy distributions, and quantitative results are obtained by Monte-Carlo simulations. The results lend insight into the character of the two-point distributions, and give quantitative estimates of the energy correlations, which are generally small.

  18. Experimental Studies of Prompt Fission Neutron Energy Spectra

    NASA Astrophysics Data System (ADS)

    Sardet, A.; Granier, T.; Laurent, B.; Oberstedt, A.

    Prompt fission neutron spectra were measured in the reactions 238U(n,f), 235U(n,f) and 237Np(n,f) at different incident neutron energies. The neutrons were detected using a coaxial doped p-terphenyl scintillation detector in coincidence with fission fragments and their time-of-flight was recorded. The properties of the neutron detector were determined and the results are presented in this work. A preliminary neutron detection efficiency was applied to data from the neutron-induced fission of 238U at En = 5.2 MeV, leading to encouraging results.

  19. T-odd angular correlations in the emission of prompt gamma rays and neutrons in nuclear fission induced by polarized neutrons

    NASA Astrophysics Data System (ADS)

    Danilyan, G. V.; Klenke, J.; Krakhotin, V. A.; Kopach, Yu. N.; Novitsky, V. V.; Pavlov, V. S.; Shatalov, P. B.

    2011-05-01

    Study of the T-odd three-vector correlation in the emission of prompt neutrons from 235U fission by polarized cold neutrons has been continued at the facility MEPHISTO of the FRM II reactor (Technical University of Munich). The sought correlation was not found within experimental error of 2.3 × 10-5. The upper limit for the asymmetry coefficient has been set to | D n | < 6 × 10-5 at 99% confidence level, whereas for ternary fission correlation coefficient D α = (170±20) × 10-5. This limit casts doubt on a model that explains the three-vector correlation in ternary fission by the Coriolis mechanism. At the same time, five-vector correlation in the emission of prompt fission neutrons has been measured, which describes the rotation of the fissioning nucleus at the moment it breaks (ROT effect). At the angle 22.5° to the fission axis, the correlation coefficient was found to be (1.57 ± 0.20) × 10-4, while at the angle of 67.5° it is zero within the experimental uncertainty. The existence of ROT effect in the emission of prompt fission neutrons can be explained by the anisotropy of neutron emission in the rest frame of the fragment (fission fragments are aligned with respect to the axis of deformation of the fissioning nucleus), similar to the mechanism of ROT effect in the emission of prompt γ-rays.

  20. Prompt Fission Neutron Spectra of Actinides

    SciTech Connect

    Capote, R; Chen, Y J; Hambsch, F J; Kornilov, N V; Lestone, J P; Litaize, O; Morillon, B; Neudecker, D; Oberstedt, S; Ohsawa, T; Smith, D. L.

    2016-01-01

    The energy spectrum of prompt neutrons emitted in fission (PFNS) plays a very important role in nuclear science and technology. A Coordinated Research Project (CRP) “Evaluation of Prompt Fission Neutron Spectra of Actinides”was established by the IAEA Nuclear Data Section in 2009, with the major goal to produce new PFNS evaluations with uncertainties for actinide nuclei. The following technical areas were addressed: (i) experiments and uncertainty quantification (UQ): New data for neutron-induced fission of 233U, 235U, 238U, and 239Pu have been measured, and older data have been compiled and reassessed. There is evidence from the experimental work of this CRP that a very small percentage of neutrons emitted in fission are actually scission neutrons; (ii) modeling: The Los Alamos model (LAM) continues to be the workhorse for PFNS evaluations. Monte Carlo models have been developed that describe the fission phenomena microscopically, but further development is needed to produce PFNS evaluations meeting the uncertainty targets; (iii) evaluation methodologies: PFNS evaluations rely on the use of the least-squares techniques for merging experimental and model data. Considerable insight was achieved on how to deal with the problem of too small uncertainties in PFNS evaluations. The importance of considering that all experimental PFNS data are “shape” data was stressed; (iv) PFNS evaluations: New evaluations, including covariance data, were generated for major actinides including 1) non-model GMA evaluations of the 235U(nth,f), 239Pu(nth,f), and 233U(nth,f) PFNS based exclusively on experimental data (0.02 ≤ E ≤ 10 MeV), which resulted in PFNS average energies E of 2.00±0.01, 2.073±0.010, and 2.030±0.013 MeV, respectively; 2) LAM evaluations of neutron-induced fission spectra on uranium and plutonium targets with improved UQ for incident energies from thermal up to 30 MeV; and 3) Point-by-Point calculations for 232Th, 234U and 237Np targets; and (v) data

  1. Prompt Neutron Lifetime for the NBSR Reactor

    SciTech Connect

    Hanson, A.L.; Diamond, D.

    2012-06-24

    In preparation for the proposed conversion of the National Institute of Standards and Technology (NIST) research reactor (NBSR) from high-enriched uranium (HEU) to low-enriched uranium (LEU) fuel, certain point kinetics parameters must be calculated. We report here values of the prompt neutron lifetime that have been calculated using three independent methods. All three sets of calculations demonstrate that the prompt neutron lifetime is shorter for the LEU fuel when compared to the HEU fuel and longer for the equilibrium end-of-cycle (EOC) condition when compared to the equilibrium startup (SU) condition for both the HEU and LEU fuels.

  2. Prompt Fission Neutron Emission in Resonance Fission of 239Pu

    NASA Astrophysics Data System (ADS)

    Hambsch, Franz-Josef; Varapai, Natallia; Zeinalov, Shakir; Oberstedt, Stephan; Serot, Olivier

    2005-05-01

    The prompt neutron emission probability from neutron-induced fission in the resonance region is being investigated at the time-of-flight facility GELINA of the IRMM. A double Frisch-gridded ionization chamber is used as a fission-fragment detector. For the data acquisition of both the fission-fragment signals as well as the neutron detector signals the fast digitization technique has been applied. For the neutron detection, large-volume liquid scintillation detectors from the DEMON collaboration are used. A specialized data analysis program taking advantage of the digital filtering technique has been developed to treat the acquired data. Neutron multiplicity investigations for actinides, especially in resonance neutron-induced fission, are rather scarce. They are, however, important for reactor control and safety issues as well as for understanding the basic physics of the fission process. Fission yield measurements on both 235U and 239Pu without prompt neutron emission coincidence have shown that fluctuation of the fission-fragment mass distribution exists from resonance to resonance, larger in the case of 235U. To possibly explain these observations, the question now is whether the prompt neutron multiplicity shows similar fluctuations with resonance energy.

  3. T-odd angular correlations in the emission of prompt gamma rays and neutrons in nuclear fission induced by polarized neutrons

    SciTech Connect

    Danilyan, G. V.; Klenke, J.; Krakhotin, V. A.; Kopach, Yu. N.; Novitsky, V. V.; Pavlov, V. S.; Shatalov, P. B.

    2011-05-15

    Study of the T-odd three-vector correlation in the emission of prompt neutrons from {sup 235}U fission by polarized cold neutrons has been continued at the facility MEPHISTO of the FRM II reactor (Technical University of Munich). The sought correlation was not found within experimental error of 2.3 Multiplication-Sign 10{sup -5}. The upper limit for the asymmetry coefficient has been set to vertical bar D{sub n} vertical bar < 6 Multiplication-Sign 10{sup -5} at 99% confidence level, whereas for ternary fission correlation coefficient D{sub {alpha}} = (170{+-}20) Multiplication-Sign 10{sup -5}. This limit casts doubt on a model that explains the three-vector correlation in ternary fission by the Coriolis mechanism. At the same time, five-vector correlation in the emission of prompt fission neutrons has been measured, which describes the rotation of the fissioning nucleus at the moment it breaks (ROT effect). At the angle 22.5 Degree-Sign to the fission axis, the correlation coefficient was found to be (1.57 {+-} 0.20) Multiplication-Sign 10{sup -4}, while at the angle of 67.5 Degree-Sign it is zero within the experimental uncertainty. The existence of ROT effect in the emission of prompt fission neutrons can be explained by the anisotropy of neutron emission in the rest frame of the fragment (fission fragments are aligned with respect to the axis of deformation of the fissioning nucleus), similar to the mechanism of ROT effect in the emission of prompt {gamma}-rays.

  4. Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances

    DOE PAGESBeta

    Neudecker, D.; Talou, P.; Kawano, T.; Smith, D. L.; Capote, R.; Rising, M. E.; Kahler, A. C.

    2015-08-01

    We present evaluations of the prompt fission neutron spectrum (PFNS) of ²³⁹Pu induced by 500 keV neutrons, and associated covariances. In a previous evaluation by Talou et al. 2010, surprisingly low evaluated uncertainties were obtained, partly due to simplifying assumptions in the quantification of uncertainties from experiment and model. Therefore, special emphasis is placed here on a thorough uncertainty quantification of experimental data and of the Los Alamos model predicted values entering the evaluation. In addition, the Los Alamos model was extended and an evaluation technique was employed that takes into account the qualitative differences between normalized model predicted valuesmore » and experimental shape data. These improvements lead to changes in the evaluated PFNS and overall larger evaluated uncertainties than in the previous work. However, these evaluated uncertainties are still smaller than those obtained in a statistical analysis using experimental information only, due to strong model correlations. Hence, suggestions to estimate model defect uncertainties are presented, which lead to more reasonable evaluated uncertainties. The calculated keff of selected criticality benchmarks obtained with these new evaluations agree with each other within their uncertainties despite the different approaches to estimate model defect uncertainties. The keff one standard deviations overlap with some of those obtained using ENDF/B-VII.1, albeit their mean values are further away from unity. Spectral indexes for the Jezebel critical assembly calculated with the newly evaluated PFNS agree with the experimental data for selected (n,γ) and (n,f) reactions, and show improvements for high-energy threshold (n,2n) reactions compared to ENDF/B-VII.1.« less

  5. Evaluation of the ²³⁹Pu prompt fission neutron spectrum induced by neutrons of 500 keV and associated covariances

    SciTech Connect

    Neudecker, D.; Talou, P.; Kawano, T.; Smith, D. L.; Capote, R.; Rising, M. E.; Kahler, A. C.

    2015-08-01

    We present evaluations of the prompt fission neutron spectrum (PFNS) of ²³⁹Pu induced by 500 keV neutrons, and associated covariances. In a previous evaluation by Talou et al. 2010, surprisingly low evaluated uncertainties were obtained, partly due to simplifying assumptions in the quantification of uncertainties from experiment and model. Therefore, special emphasis is placed here on a thorough uncertainty quantification of experimental data and of the Los Alamos model predicted values entering the evaluation. In addition, the Los Alamos model was extended and an evaluation technique was employed that takes into account the qualitative differences between normalized model predicted values and experimental shape data. These improvements lead to changes in the evaluated PFNS and overall larger evaluated uncertainties than in the previous work. However, these evaluated uncertainties are still smaller than those obtained in a statistical analysis using experimental information only, due to strong model correlations. Hence, suggestions to estimate model defect uncertainties are presented, which lead to more reasonable evaluated uncertainties. The calculated keff of selected criticality benchmarks obtained with these new evaluations agree with each other within their uncertainties despite the different approaches to estimate model defect uncertainties. The keff one standard deviations overlap with some of those obtained using ENDF/B-VII.1, albeit their mean values are further away from unity. Spectral indexes for the Jezebel critical assembly calculated with the newly evaluated PFNS agree with the experimental data for selected (n,γ) and (n,f) reactions, and show improvements for high-energy threshold (n,2n) reactions compared to ENDF/B-VII.1.

  6. Searches for T-odd correlations in the emission of prompt neutrons in the polarized-neutron-induced fission of 235U nuclei

    NASA Astrophysics Data System (ADS)

    Danilyan, G. V.; Klenke, J.; Krakhotin, V. A.; Novitsky, V. V.; Pavlov, V. S.; Shatalov, P. B.

    2010-07-01

    The results of an experiment aimed at searches for formally T-odd correlations in the angular distribution of prompt neutrons from the fission of 235U nuclei are presented. The experiment was performed in the MEPHISTO polarized cold-neutron beam from the Munich FRMII reactor. The correlation coefficient proved to be (-3.5 ± 3.4) × 10-5 for a three-vector correlation (TRI effect) and (-5.0 ± 3.4) × 10-5 for a five-vector correlation (ROT effect). This means that no significant effects were discovered within the measurement errors. A comparison with the analogous effects in the ternary fission of 235U nuclei was performed. The values of the corresponding correlations in the angular distribution of prompt fission gamma rays were refined.

  7. The Need for Precise and Well-documented Experimental Data on Prompt Fission Neutron Spectra from Neutron-induced Fission of 239Pu

    NASA Astrophysics Data System (ADS)

    Neudecker, D.; Taddeucci, T. N.; Haight, R. C.; Lee, H. Y.; White, M. C.; Rising, M. E.

    2016-01-01

    The spectrum of neutrons emitted promptly after 239Pu(n,f)-a so-called prompt fission neutron spectrum (PFNS)-is a quantity of high interest, for instance, for reactor physics and global security. However, there are only few experimental data sets available that are suitable for evaluations. In addition, some of those data sets differ by more than their 1-σ uncertainty boundaries. We present the results of MCNP studies indicating that these differences are partly caused by underestimated multiple scattering contributions, over-corrected background, and inconsistent deconvolution methods. A detailed uncertainty quantification for suitable experimental data was undertaken including these effects, and test-evaluations were performed with the improved uncertainty information. The test-evaluations illustrate that the inadequately estimated effects and detailed uncertainty quantification have an impact on the evaluated PFNS and associated uncertainties as well as the neutron multiplicity of selected critical assemblies. A summary of data and documentation needs to improve the quality of the experimental database is provided based on the results of simulations and test-evaluations. Given the possibly substantial distortion of the PFNS by multiple scattering and background effects, special care should be taken to reduce these effects in future measurements, e.g., by measuring the 239Pu PFNS as a ratio to either the 235U or 252Cf PFNS.

  8. The need for precise and well-documented experimental data on prompt fission neutron spectra from neutron-induced fission of 239Pu

    DOE PAGESBeta

    Neudecker, Denise; Taddeucci, Terry Nicholas; Haight, Robert Cameron; Lee, Hye Young; White, Morgan Curtis; Rising, Michael Evans

    2016-01-06

    The spectrum of neutrons emitted promptly after 239Pu(n,f)—a so-called prompt fission neutron spectrum (PFNS)—is a quantity of high interest, for instance, for reactor physics and global security. However, there are only few experimental data sets available that are suitable for evaluations. In addition, some of those data sets differ by more than their 1-σ uncertainty boundaries. We present the results of MCNP studies indicating that these differences are partly caused by underestimated multiple scattering contributions, over-corrected background, and inconsistent deconvolution methods. A detailed uncertainty quantification for suitable experimental data was undertaken including these effects, and test-evaluations were performed with themore » improved uncertainty information. The test-evaluations illustrate that the inadequately estimated effects and detailed uncertainty quantification have an impact on the evaluated PFNS and associated uncertainties as well as the neutron multiplicity of selected critical assemblies. A summary of data and documentation needs to improve the quality of the experimental database is provided based on the results of simulations and test-evaluations. Furthermore, given the possibly substantial distortion of the PFNS by multiple scattering and background effects, special care should be taken to reduce these effects in future measurements, e.g., by measuring the 239Pu PFNS as a ratio to either the 235U or 252Cf PFNS.« less

  9. Prompt neutron multiplicities for the transplutonium nuclides

    SciTech Connect

    Holden, N.E.; Zucker, M.S.

    1985-01-01

    The direct determination of the average prompt neutron emission values is reviewed, and a method of comparing different sites of neutron emission multiplicity distribution values is described. Measured and recommended values are tabulated for these nuclides: /sup 241/Am, /sup 242/Am, /sup 242/Cm, /sup 243/Cm, /sup 244/Cm, /sup 246/Cm, /sup 247/Cm, /sup 248/Cm, /sup 250/Cm, /sup 245/Cm, /sup 249/Bk, /sup 246/Cf, /sup 249/Cf, /sup 250/Cf, /sup 252/Cf, /sup 254/Cf, /sup 251/Cf, /sup 253/Es, /sup 254/Es, /sup 244/Fm, /sup 246/Fm, /sup 255/Fm, /sup 252/No, /sup 254/Fm, /sup 256/Fm, /sup 257/Fm. 59 refs., 24 tabs. (LEW)

  10. Introducing Nuclear Data Evaluations of Prompt Fission Neutron Spectra

    SciTech Connect

    Neudecker, Denise

    2015-06-17

    Nuclear data evaluations provide recommended data sets for nuclear data applications such as reactor physics, stockpile stewardship or nuclear medicine. The evaluated data are often based on information from multiple experimental data sets and nuclear theory using statistical methods. Therefore, they are collaborative efforts of evaluators, theoreticians, experimentalists, benchmark experts, statisticians and application area scientists. In this talk, an introductions is given to the field of nuclear data evaluation at the specific example of a recent evaluation of the outgoing neutron energy spectrum emitted promptly after fission from 239Pu and induced by neutrons from thermal to 30 MeV.

  11. Effects of rotation of fissioning nuclei in the angular distributions of prompt neutrons and gamma rays originating from the polarized-neutron-induced fission of 233U and 235U nuclei

    NASA Astrophysics Data System (ADS)

    Danilyan, G. V.; Klenke, J.; Kopach, Yu. N.; Krakhotin, V. A.; Novitsky, V. V.; Pavlov, V. S.; Shatalov, P. B.

    2014-06-01

    The results of an experiment devoted to searches for effects of rotation of fissioning nuclei in the angular distributions of prompt neutrons and gamma rays originating from the polarized-neutron-induced fission of 233U nuclei are presented. The effects discovered in these angular distributions are opposite in sign to their counterparts in the polarized-neutron-induced fission of 235U nuclei. This is at odds with data on the relative signs of respective effects in the angular distribution of alpha particles from the ternary fission of the same nuclei and may be indicative of problems in the model currently used to describe the effect in question. The report on which this article is based was presented at the seminar held at the Institute of Theoretical and Experimental Physics and dedicated to the 90th anniversary of the birth of Yu.G. Abov, corresponding member of Russian Academy of Sciences, Editor in Chief of the journal Physics of Atomic Nuclei.

  12. Physical basis for prompt-neutron activation analysis

    SciTech Connect

    Chrien, R.E.

    1982-01-01

    The technique called prompt ..gamma..-ray neutron activation analysis has been applied to rapid materials analysis. The radiation following the neutron radiation capture is prompt in the sense that the nuclear decay time is on the order of 10/sup -15/ second, and thus the technique is not strictly activation, but should be called radiation neutron capture spectroscopy or neutron capture ..gamma..-ray spectroscopy. This paper reviews the following: sources and detectors, theory of radiative capture, nonstatistical capture, giant dipole resonance, fast neutron capture, and thermal neutron capture ..gamma..-ray spectra. 14 figures.

  13. Use of prompt gamma emissions from polyethylene to estimate neutron ambient dose equivalent

    NASA Astrophysics Data System (ADS)

    Priyada, P.; Sarkar, P. K.

    2015-06-01

    The possibility of using measured prompt gamma emissions from polyethylene to estimate neutron ambient dose equivalent is explored theoretically. Monte Carlo simulations have been carried out using the FLUKA code to calculate the response of a high density polyethylene cylinder to emit prompt gammas from interaction of neutrons with the nuclei of hydrogen and carbon present in polyethylene. The neutron energy dependent responses of hydrogen and carbon nuclei are combined appropriately to match the energy dependent neutron fluence to ambient dose equivalent conversion coefficients. The proposed method is tested initially with simulated spectra and then validated using experimental measurements with an Am-Be neutron source. Experimental measurements and theoretical simulations have established the feasibility of estimating neutron ambient dose equivalent using measured neutron induced prompt gammas emitted from polyethylene with an overestimation of neutron dose at very low energies.

  14. Detection of thermal-induced prompt fission neutrons of highly-enriched uranium: A position sensitive technique

    NASA Astrophysics Data System (ADS)

    Tartaglione, A.; Di Lorenzo, F.; Mayer, R. E.

    2009-07-01

    Cargo interrogation in search for special nuclear materials like highly-enriched uranium or 239Pu is a first priority issue of international borders security. In this work we present a thermal-pulsed neutron-based approach to a technique which combines the time-of-flight method and demonstrates a capability to detect small quantities of highly-enriched uranium shielded with high or low Z materials providing, in addition, a manner to know the approximate position of the searched material.

  15. Imaging and Radiography with Nuclear Resonance Fluorescence and Effective-Z (EZ-3D) Determination; SNM Detection Using Prompt Neutrons from Photon Induced Fission

    SciTech Connect

    Bertozzi, William; Hasty, Richard; Klimenko, Alexei; Korbly, Stephen E.; Ledoux, Robert J.; Park, William

    2009-03-10

    Four new technologies have been developed for use in non-intrusive inspection systems to detect nuclear materials, explosives and contraband. Nuclear Resonance Fluorescence (NRF) provides a three dimensional image of the isotopic content of a container. NRF determines the isotopic composition of a region and specifies the isotopic structure of the neighboring regions, thus providing the detailed isotopic composition of any threat. In transmission mode, NRF provides a two dimensional projection of the isotopic content of a container, much as standard X-ray radiography provides for density. The effective-Z method (EZ-3D) uses electromagnetic scattering processes to yield a three-dimensional map of the effective-Z and the density in a container. The EZ-3D method allows for a rapid discrimination based on effective Z and mass of materials such as those with high Z, as well as specifying regions of interest for other contraband. The energy spectrum of prompt neutrons from photon induced fission (PNPF) provides a unique identification of the presence of actinides and SNM. These four new technologies can be used independently or together to automatically determine the presence of hazardous materials or contraband. They can also be combined with other technologies to provide added specificity.

  16. Imaging and Radiography with Nuclear Resonance Fluorescence and Effective-Z (EZ-3D™) Determination; SNM Detection Using Prompt Neutrons from Photon Induced Fission

    NASA Astrophysics Data System (ADS)

    Bertozzi, William; Hasty, Richard; Klimenko, Alexei; Korbly, Stephen E.; Ledoux, Robert J.; Park, William

    2009-03-01

    Four new technologies have been developed for use in non-intrusive inspection systems to detect nuclear materials, explosives and contraband. Nuclear Resonance Fluorescence (NRF) provides a three dimensional image of the isotopic content of a container. NRF determines the isotopic composition of a region and specifies the isotopic structure of the neighboring regions, thus providing the detailed isotopic composition of any threat. In transmission mode, NRF provides a two dimensional projection of the isotopic content of a container, much as standard X-ray radiography provides for density. The effective-Z method (EZ-3D™) uses electromagnetic scattering processes to yield a three-dimensional map of the effective-Z and the density in a container. The EZ-3D™ method allows for a rapid discrimination based on effective Z and mass of materials such as those with high Z, as well as specifying regions of interest for other contraband. The energy spectrum of prompt neutrons from photon induced fission (PNPF) provides a unique identification of the presence of actinides and SNM. These four new technologies can be used independently or together to automatically determine the presence of hazardous materials or contraband. They can also be combined with other technologies to provide added specificity.

  17. A new approach to prompt fission neutron TOF data treatment

    NASA Astrophysics Data System (ADS)

    Zeynalov, Sh.; Zeynalova, O. V.; Hambsch, F.-J.; Oberstedt, S.

    The prompt neutron emission in spontaneous fission of 252Cf has been investigated applying digital signal electronics along with associated digital signal processing algorithms. A new mathematical approach, applicable to single events, was developed for prompt fission neutron (PFN) time-offlight distribution unfolding. The main goal was to understand the reasons of the long existing discrepancy between theoretical calculations and the measurements of prompt fission neutron (PFN) emission dependence on the total kinetic energy (TKE) of the fission fragments (FF). Since the 252Cf (sf) reaction is one of the main references for nuclear data the understanding of the PFN emission mechanism is very important both for nuclear fission theory and nuclear data. The experimental data were taken with a twin Frisch-grid ionization chamber and a NE213-equivalent neutron detector in an experimental setup similar to the well known work of C. Budtz-Jorgensen and H.-H. Knitter. About 2.5 × 105 coincidences between fission fragment (FF) and neutron detector response to prompt fission neutron detection have been registered (∼ 1.6 × 107 of total recorded fission events). Fission fragment kinetic energy, mass and angular distribution, neutron time-of-flight and pulse shape have been investigated using a 12-bit waveform digitizer. The signal waveforms have been analyzed using digital signal processing algorithms. The main goal of this work was a detailed description of the prompt fission neutron treatment.

  18. Prompt neutron multiplicity measurements with portable detectors

    NASA Astrophysics Data System (ADS)

    Mukhopadhyay, Sanjoy; Wolff, Ronald; Maurer, Richard; Mitchell, Stephen; Smith, Ethan X.; Guss, Paul; Lacy, Jeffrey L.; Sun, L.; Athanasiades, A.

    2011-09-01

    Mobile detection of kilogram quantities of special nuclear materials (SNM) during maritime transportation is a challenging problem for the U.S. Department of Homeland Security. Counting neutrons emitted by the SNM and partitioning them from background neutrons of multiple origins is the most effective passive means of detecting the SNM. Unfortunately, neutron detection, counting, and partitioning in a maritime environment is complex due to the presence of spallation neutrons (commonly known as "ship effect") and to the complicated nature of the neutron scattering in that environment. This work studied the possibilities of building a prototype neutron detector using boron- 10 (10B) as the converter in a novel form factor called "straws" that would address the above problem by examining multiplicity distributions of neutrons originating from a fissioning source. Currently, commercially manufactured fission meters (FM) are available that separate cosmic neutrons from non-cosmic neutrons and quantitatively determine the strength of a fissioning source; however, these FMs use 3He, which is becoming increasingly difficult to procure; also the size and weight of a commercial FM is not conducive to manual neutron detection operations in a maritime environment. The current project may provide a near-term solution to the crisis that has arisen from the global scarcity of 3He by offering a viable alternative to the FM. The prototype detector provides a large-area, efficient, lightweight, more granular neutron responsive detection surface (to facilitate imaging) to ease the application of the new FMs.

  19. Cross correlation method application to prompt fission neutron investigation

    NASA Astrophysics Data System (ADS)

    Zeynalova, O. V.; Zeynalov, Sh.; Nazarenko, M. A.; Hambsch, F.-J.; Oberstedt, S.

    2012-10-01

    Do The prompt neutron emission in spontaneous fission of 252Cf has been investigated applying cross correlation method and digital signal processing algorithms. A new mathematical approach for neutron/gamma pulse shape separation was developed and implemented for prompt fission neutron (PFN) time-of-flight measurement. The main goal was development of automated data analysis algorithms and procedures for data analysis with minimum human intervention. Experimental data was taken with a twin Frisch-grid ionization chamber and a NE213-equivalent neutron detector in an experimental setup similar to well work of C. Budtz-Jorgensen and H.-H. Knitter [1]. About 2*107 fission events were registered with 2*105 neutron/gamma detection in coincidence with fission fragments. Fission fragment kinetic energy, mass and angular distribution, neutron time-of-flight and pulse shape have been investigated using a 12 bit waveform digitizer.

  20. Prompt Neutron Multiplicity Measurements with Portable Detectors

    SciTech Connect

    S. Mukhopadhyay, R. Wolff, R. Maurer, S. Mitchell, E. X. Smith, P. Guss, J. L. Lacy, L. Sun, A. Athanasiades

    2011-09-01

    Mobile detection of kilogram quantities of special nuclear materials (SNM) during maritime transportation is a challenging problem for the U.S. Department of Homeland Security. Counting neutrons emitted by the SNM and partitioning them from background neutrons of multiple origins is the most effective passive means of detecting the SNM. Unfortunately, neutron detection, counting, and partitioning in a maritime environment is complex due to the presence of spallation neutrons (commonly known as “ship effect”) and to the complicated nature of the neutron scattering in that environment. This work studied the possibilities of building a prototype neutron detector using boron- 10 (10B) as the converter in a novel form factor called “straws” that would address the above problem by examining multiplicity distributions of neutrons originating from a fissioning source. Currently, commercially manufactured fission meters (FM) are available that separate cosmic neutrons from non-cosmic neutrons and quantitatively determine the strength of a fissioning source; however, these FMs use 3He, which is becoming increasingly difficult to procure; also the size and weight of a commercial FM is not conducive to manual neutron detection operations in a maritime environment. The current project may provide a near-term solution to the crisis that has arisen from the global scarcity of 3He by offering a viable alternative to the FM. The prototype detector provides a large-area, efficient, lightweight, more granular neutron responsive detection surface (to facilitate imaging) to ease the application of the new FMs. A novel prototype fission meter is being designed at National Security Technologies, LLC, using a thin uniform coating of 10B as neutron converter (only 1 micron thick) inside a large array of thin (4 mm diameter) copper tubes. The copper tubes are only 2-mil thick, and each holds the stretched anode wire under tension and high voltage. The tubes are filled with

  1. Isotope identification capabilities using time resolved prompt gamma emission from epithermal neutrons

    NASA Astrophysics Data System (ADS)

    Festa, G.; Arcidiacono, L.; Pappalardo, A.; Minniti, T.; Cazzaniga, C.; Scherillo, A.; Andreani, C.; Senesi, R.

    2016-03-01

    We present a concept of integrated measurements for isotope identification which takes advantage of the time structure of spallation neutron sources for time resolved γ spectroscopy. Time resolved Prompt Gamma Activation Analysis (T-PGAA) consists in the measurement of gamma energy spectrum induced by the radioactive capture as a function of incident neutron Time Of Flight (TOF), directly related with the energy of incident neutrons. The potential of the proposed concept was explored on INES (Italian Neutron Experimental Station) at the ISIS spallation neutron source (U.K.). Through this new technique we show an increase in the sensitivity to specific elements of archaeometric relevance, through incident neutron energy selection in prompt γ spectra for multicomponent samples. Results on a standard bronze sample are presented.

  2. Prompt Fission Neutron Experiments on 235U(n,f) and 252Cf(SF)

    NASA Astrophysics Data System (ADS)

    Göök, A.; Hambsch, F.-J.; Oberstedt, S.; Vidali, M.

    For nuclear modeling and improved evaluation of nuclear data knowledge about fluctuations of the prompt neutron multiplicity as a function of incident neutron energy is requested for the major actinides 235U and 239Pu. Experimental investigations of the prompt fission neutron emission in resonance neutron induced fission on 235U are taking place at the GELINA facility of the IRMM. The experiment employs an array of neutron scintillation-detectors (SCINTIA) in conjunction with a newly designed 3D position sensitive twin Frisch-grid ionization chamber. A preparatory experiment on prompt fission neutron emission in 252Cf(SF) was undertaken to verify analysis procedures relevant for the implementation of the SCINTIA neutron detector array. The available literature data on the TKE dependence of the multiplicity show strong deviations. Therefore, effort was focused on investigating experimental factors in low efficiency neutron counting experiments that may lead to faulty determination of this dependence. Taking these factors into account a result that agree well with data from high efficiency neutron counting experiments is obtained.

  3. A New Method of Prompt Fission Neutron Energy Spectrum Unfolding

    NASA Astrophysics Data System (ADS)

    Zeynalova, O. V.; Zeynalov, Sh.; Hambsch, F.-J.; Oberstedt, S.

    2010-11-01

    The prompt neutron emission in spontaneous fission of 252Cf has been investigated applying digital signal electronics along with associated digital signal processing algorithms. The goal was to find out the reasons of a long time existing discrepancy between theoretical calculations and the measurements of prompt fission neutron (PFN) emission dependence on the total kinetic energy (TKE) of fission fragments (FF). On the one hand the 252Cf (sf) reaction is one of the main references for nuclear data, on the other hand the understanding of PFN emission mechanism is very important for nuclear fission theory. Using a twin Frisch-grid ionization chamber for fission fragment (FF) detection and a NE213-equivalent neutron detector in total about 107 fission fragment-neutron coincidences have been registered. Fission fragment kinetic energy, mass and angular distribution, neutron time-of-flight and pulse shape have been investigated using a 12 bit waveform digitizer. The signal waveforms have been analyzed using digital signal processing algorithms. For the first time the dependence of the number of emitted neutrons as a function of total kinetic energy (TKE) of the fragments is in very good agreement with theoretical calculations in the range of TKE from 140-220 MeV.

  4. A New Method of Prompt Fission Neutron Energy Spectrum Unfolding

    SciTech Connect

    Zeynalova, O. V.; Zeynalov, Sh.; Hambsch, F.-J.; Oberstedt, S.

    2010-11-25

    The prompt neutron emission in spontaneous fission of {sup 252}Cf has been investigated applying digital signal electronics along with associated digital signal processing algorithms. The goal was to find out the reasons of a long time existing discrepancy between theoretical calculations and the measurements of prompt fission neutron (PFN) emission dependence on the total kinetic energy (TKE) of fission fragments (FF). On the one hand the {sup 252}Cf(sf) reaction is one of the main references for nuclear data, on the other hand the understanding of PFN emission mechanism is very important for nuclear fission theory. Using a twin Frisch-grid ionization chamber for fission fragment (FF) detection and a NE213-equivalent neutron detector in total about 10{sup 7} fission fragment-neutron coincidences have been registered. Fission fragment kinetic energy, mass and angular distribution, neutron time-of-flight and pulse shape have been investigated using a 12 bit waveform digitizer. The signal waveforms have been analyzed using digital signal processing algorithms. For the first time the dependence of the number of emitted neutrons as a function of total kinetic energy (TKE) of the fragments is in very good agreement with theoretical calculations in the range of TKE from 140-220 MeV.

  5. The LANL/LLNL Prompt Fission Neutron Spectrum Program at LANSCE and Approach to Uncertainties

    SciTech Connect

    Haight, R.C.; Wu, C.Y.; Lee, H.Y.; Taddeucci, T.N.; Perdue, B.A.; O'Donnell, J.M.; Fotiades, N.; Devlin, M.; Ullmann, J.L.; Bredeweg, T.A.; Jandel, M.; Nelson, R.O.; Wender, S.A.; Neudecker, D.; Rising, M.E.; Mosby, S.; Sjue, S.; White, M.C.; Bucher, B.; Henderson, R.

    2015-01-15

    New data on the prompt fission neutron spectra (PFNS) from neutron-induced fission with higher accuracies are needed to resolve discrepancies in the literature and to address gaps in the experimental data. The Chi-Nu project, conducted jointly by LANL and LLNL, aims to measure the shape of the PFNS for fission of {sup 239}Pu induced by neutrons from 0.5 to 20 MeV with accuracies of 3–5% in the outgoing energy from 0.1 to 9 MeV and 15% from 9 to 12 MeV and to provide detailed experimental uncertainties. Neutrons from the WNR/LANSCE neutron source are being used to induce fission in a Parallel-Plate Avalanche Counter (PPAC). Two arrays of neutron detectors are used to cover the energy range of neutrons emitted promptly in the fission process. Challenges for the present experiment include background reduction, use of {sup 239}Pu in a PPAC, and understanding neutron detector response. Achieving the target accuracies requires the understanding of many systematic uncertainties. The status and plans for the future will be presented.

  6. Effective delayed neutron fraction and prompt neutron lifetime of Tehran research reactor mixed-core.

    PubMed

    Lashkari, A; Khalafi, H; Kazeminejad, H

    2013-05-01

    In this work, kinetic parameters of Tehran research reactor (TRR) mixed cores have been calculated. The mixed core configurations are made by replacement of the low enriched uranium control fuel elements with highly enriched uranium control fuel elements in the reference core. The MTR_PC package, a nuclear reactor analysis tool, is used to perform the analysis. Simulations were carried out to compute effective delayed neutron fraction and prompt neutron lifetime. Calculation of kinetic parameters is necessary for reactivity and power excursion transient analysis. The results of this research show that effective delayed neutron fraction decreases and prompt neutron lifetime increases with the fuels burn-up. Also, by increasing the number of highly enriched uranium control fuel elements in the reference core, the prompt neutron lifetime increases, but effective delayed neutron fraction does not show any considerable change. PMID:24976672

  7. Impact of prompt-neutron corrections on final fission-fragment distributions

    NASA Astrophysics Data System (ADS)

    Al-Adili, A.; Hambsch, F.-J.; Pomp, S.; Oberstedt, S.

    2012-11-01

    Background: One important quantity in nuclear fission is the average number of prompt neutrons emitted from the fission fragments, the prompt neutron multiplicity, ν¯. The total number of prompt fission neutrons, ν¯tot, increases with increasing incident neutron energy. The prompt-neutron multiplicity is also a function of the fragment mass and the total kinetic energy of the fragmentation. Those data are only known in sufficient detail for a few thermal-neutron-induced fission reactions on, for example, 233,235U and 239Pu. The enthralling question has always been asked how the additional excitation energy is shared between the fission fragments. The answer to this question is important in the analysis of fission-fragment data taken with the double-energy technique. Although in the traditional approach the excess neutrons are distributed equally across the mass distribution, a few experiments showed that those neutrons are predominantly emitted by the heavy fragments.Purpose: We investigated the consequences of the ν(A,TKE,En) distribution on the fission fragment observables.Methods: Experimental data obtained for the 234U(n,f) reaction with a Twin Frisch Grid Ionization Chamber, were analyzed assuming two different methods for the neutron evaporation correction. The effect of the two different methods on the resulting fragment mass and energy distributions is studied.Results: We found that the preneutron mass distributions obtained via the double-energy technique become slightly more symmetric, and that the impact is larger for postneutron fission-fragment distributions. In the most severe cases, a relative yield change up to 20-30% was observed.Conclusions: We conclude that the choice of the prompt-neutron correction method has strong implications on the understanding and modeling of the fission process and encourages new experiments to measure fission fragments in coincidence with prompt fission neutrons. Even more, the correct determination of postneutron

  8. Testing The High-Energy Prompt Neutron Signature At Low Beam Energies

    SciTech Connect

    Thompson, Scott J.; Kinlaw, Mathew T.; Hunt, Alan W.

    2011-06-01

    Prompt fission neutrons continue to be examined as a signature for detecting the presence of fissionable material. This technique exploits the neutron energy limitations inherent with photonuclear emissions from non-fissionable material, allowing prompt fission neutrons to be identified and engaged for detecting nuclear material. Prompt neutron signal measurements were acquired with bremsstrahlung endpoint energies of 6 MeV for 18 targets comprised of both fissionable and non-fissionable material; delayed neutron measurements were also collected as a reference. The {sup 238}U target was also shielded with increasing thicknesses of lead or borated polyethylene to compare the resulting detection rates of the prompt and delayed fission neutron signals.

  9. Prompt Neutron Emission in 252CF Spontaneous Fission

    NASA Astrophysics Data System (ADS)

    Hambsch, F.-J.; Oberstedt, S.; Zeynalov, Sh.

    2011-10-01

    The prompt neutron emission in spontaneous fission of 252Cf has been investigated applying digital signal electronics. The goal was to compare the results from digital data acquisition and digital signal processing analysis with results of the pioneering work of Budtz-Jørgensen and Knitter. Using a twin Frisch-grid ionization chamber for fission fragment (FF) detection and a NE213-equivalent neutron detector in total about 107 fission fragment-neutron coincidences have been registered. Fission fragment kinetic energy, mass and angular distribution, neutron time-of-flight and pulse shape have been investigated using a 12 bit waveform digitizer. The signal waveforms have been analyzed using digital signal processing algorithms. The results are in very good agreement with literature. For the first time the dependence of the number of emitted neutrons as a function of total kinetic energy (TKE) of the fragments is in very good agreement with theoretical calculations in the range of TKE from 140-220 MeV.

  10. Prompt merger collapse and the maximum mass of neutron stars.

    PubMed

    Bauswein, A; Baumgarte, T W; Janka, H-T

    2013-09-27

    We perform hydrodynamical simulations of neutron-star mergers for a large sample of temperature-dependent nuclear equations of state and determine the threshold mass above which the merger remnant promptly collapses to form a black hole. We find that, depending on the equation of state, the threshold mass is larger than the maximum mass of a nonrotating star in isolation by between 30 and 70 percent. Our simulations also show that the ratio between the threshold mass and maximum mass is tightly correlated with the compactness of the nonrotating maximum-mass configuration. We speculate on how this relation can be used to derive constraints on neutron-star properties from future observations. PMID:24116763

  11. DSP Algorithms for Fission Fragment and Prompt Fission Neutron Spectroscopy

    NASA Astrophysics Data System (ADS)

    Zeynalova, O.; Zeynalov, Sh.; Hambsch, F.-J.; Oberstedt, S.; Fabry, I.

    2009-10-01

    Digital signal processing (DSP) algorithms are in high demand for modern nuclear fission investigation due to importance of increase the accuracy of fissile nuclear data for new generation of nuclear power stations. DSP algorithms for fission fragment (FF) and prompt fission neutron (PFN) spectroscopy are described in the present work. The twin Frisch-grid ionization chamber (GTIC) is used to measure the kinetic energy-, mass- and angular distributions of the FF in the 252Cf(SF) reaction. Along with the neutron time-of-flight (TOF) measurement the correlation between neutron emission and FF mass and energy is investigated. The TOF is measured between common cathode of the GTIC and the neutron detector (ND) pulses. Waveform digitizers (WFD) having 12 bit amplitude resolution and 100 MHz sampling frequency are used for the detector pulse sampling. DSP algorithms are developed as recursive procedures to perform the signal processing, similar to those available in various nuclear electronics modules, such as constant fraction discriminator (CFD), pulse shape discriminator (PSD), peak-sensitive analogue-to-digital converter (pADC) and pulse shaping amplifier (PSA). To measure the angle between FF and the cathode plane normal to the GTIC a new algorithm is developed having advantage over the traditional analogue pulse processing schemes. Algorithms are tested by comparing the numerical simulation of the data analysis of the 252Cf(SF) reaction with data available from literature.

  12. DSP Algorithms for Fission Fragment and Prompt Fission Neutron Spectroscopy

    SciTech Connect

    Zeynalova, O.; Zeynalov, Sh.; Hambsch, F.-J.; Oberstedt, S.; Fabry, I.

    2009-10-29

    Digital signal processing (DSP) algorithms are in high demand for modern nuclear fission investigation due to importance of increase the accuracy of fissile nuclear data for new generation of nuclear power stations. DSP algorithms for fission fragment (FF) and prompt fission neutron (PFN) spectroscopy are described in the present work. The twin Frisch-grid ionization chamber (GTIC) is used to measure the kinetic energy-, mass- and angular distributions of the FF in the {sup 252}Cf(SF) reaction. Along with the neutron time-of-flight (TOF) measurement the correlation between neutron emission and FF mass and energy is investigated. The TOF is measured between common cathode of the GTIC and the neutron detector (ND) pulses. Waveform digitizers (WFD) having 12 bit amplitude resolution and 100 MHz sampling frequency are used for the detector pulse sampling. DSP algorithms are developed as recursive procedures to perform the signal processing, similar to those available in various nuclear electronics modules, such as constant fraction discriminator (CFD), pulse shape discriminator (PSD), peak-sensitive analogue-to-digital converter (pADC) and pulse shaping amplifier (PSA). To measure the angle between FF and the cathode plane normal to the GTIC a new algorithm is developed having advantage over the traditional analogue pulse processing schemes. Algorithms are tested by comparing the numerical simulation of the data analysis of the {sup 252}Cf(SF) reaction with data available from literature.

  13. RADSAT Benchmarks for Prompt Gamma Neutron Activation Analysis Measurements

    SciTech Connect

    Burns, Kimberly A.; Gesh, Christopher J.

    2011-07-01

    The accurate and efficient simulation of coupled neutron-photon problems is necessary for several important radiation detection applications. Examples include the detection of nuclear threats concealed in cargo containers and prompt gamma neutron activation analysis for nondestructive determination of elemental composition of unknown samples. High-resolution gamma-ray spectrometers are used in these applications to measure the spectrum of the emitted photon flux, which consists of both continuum and characteristic gamma rays with discrete energies. Monte Carlo transport is the most commonly used simulation tool for this type of problem, but computational times can be prohibitively long. This work explores the use of multi-group deterministic methods for the simulation of coupled neutron-photon problems. The main purpose of this work is to benchmark several problems modeled with RADSAT and MCNP to experimental data. Additionally, the cross section libraries for RADSAT are updated to include ENDF/B-VII cross sections. Preliminary findings show promising results when compared to MCNP and experimental data, but also areas where additional inquiry and testing are needed. The potential benefits and shortcomings of the multi-group-based approach are discussed in terms of accuracy and computational efficiency.

  14. Coincidence Prompt Gamma-Ray Neutron Activation Analysis

    SciTech Connect

    R.P. gandner; C.W. Mayo; W.A. Metwally; W. Zhang; W. Guo; A. Shehata

    2002-11-10

    The normal prompt gamma-ray neutron activation analysis for either bulk or small beam samples inherently has a small signal-to-noise (S/N) ratio due primarily to the neutron source being present while the sample signal is being obtained. Coincidence counting offers the possibility of greatly reducing or eliminating the noise generated by the neutron source. The present report presents our results to date on implementing the coincidence counting PGNAA approach. We conclude that coincidence PGNAA yields: (1) a larger signal-to-noise (S/N) ratio, (2) more information (and therefore better accuracy) from essentially the same experiment when sophisticated coincidence electronics are used that can yield singles and coincidences simultaneously, and (3) a reduced (one or two orders of magnitude) signal from essentially the same experiment. In future work we will concentrate on: (1) modifying the existing CEARPGS Monte Carlo code to incorporate coincidence counting, (2) obtaining coincidence schemes for 18 or 20 of the common elements in coal and cement, and (3) optimizing the design of a PGNAA coincidence system for the bulk analysis of coal.

  15. The LANL/LLNL Program to Measure Prompt Fission Neutron Spectra at LANSCE

    NASA Astrophysics Data System (ADS)

    Haight, Robert; Wu, Ching Yen; Lee, Hye Young; Taddeucci, Terry; Mosby, Shea; O'Donnell, John; Fotiades, Nikolaos; Devlin, Mattew; Ullmann, John; Nelson, Ronald; Wender, Stephen; White, Morgan; Solomon, Clell; Neudecker, Denise; Talou, Patrick; Rising, Michael; Bucher, Brian; Buckner, Matthew; Henderson, Roger

    2015-10-01

    Accurate data on the spectrum of neutrons emitted in neutron-induced fission are needed for applications and for a better understanding of the fission process. At LANSCE we have made important progress in understanding systematic uncertainties and in obtaining data for 235U on the low-energy part of the prompt fission neutron spectra (PFNS), a particularly difficult region because down-scattered neutrons go in this direction. We use a double time-of-flight technique to determine energies of incoming and outgoing neutrons. With data acquisition via waveform digitizers, accidental coincidences between fission chamber and neutron detector are measured to high statistical accuracy and then subtracted from measured events. Monte Carlo simulations with high performance computers have proven to be essential in the design to minimize neutron scattering and in calculating detector response. Results from one of three approaches to analyzing the data will be presented. This work is funded by the US Department of Energy, National Nuclear Security Administration and Office of Nuclear Physics.

  16. Absorbed Dose Rates in Tissue from Prompt Gamma Emissions from Near-thermal Neutron Absorption.

    PubMed

    Schwahn, Scott O

    2015-10-01

    Prompt gamma emission data from the International Atomic Energy Agency's Prompt Gamma-ray Neutron Activation Analysis database are analyzed to determine the absorbed dose rates in tissue to be expected when natural elements are exposed in a near-thermal neutron environment. PMID:26313590

  17. Absorbed dose rates in tissue from prompt gamma emissions from near-thermal neutron absorption

    DOE PAGESBeta

    Schwahn, Scott O.

    2015-10-01

    Prompt gamma emission data from the International Atomic Energy Agency s Prompt Gamma-ray Neutron Activation Analysis database are analyzed to determine the absorbed dose rates in tissue to be expected when natural elements are exposed in a near-thermal neutron environment.

  18. Energy measurement of prompt fission neutrons in 239Pu(n,f) for incident neutron energies from 1 to 200 MeV

    SciTech Connect

    Haight, Robert C; Devlin, Matthew J; Nelson, Ronald O; O' Donnell, John M; Chatillon, Audrey; Granier, Thierry; Taieb, Julien; Belier, Gilbert; Laurent, Benoit; Noda, Shusaku

    2010-01-01

    An experimental campaign was started in 2002 in the framework of a collaboration belween CEA-DAM and the Los Alamos National Laboratory to measure the prompt fission neutron spectra (PFNS) for incident neutron energies from 1 to 200 MeV with consistent error uncertainties over the whole energy range. The prompt neutron spectra in {sup 235,238}U(n,f) and {sup 237}Np(n,f) have been already studied successfully. A first attempt to characterize the prompt neutrons emitted during the fission of the {sup 239}Pu was done in 2007. This contribution will focus on the results obtained during the final experiment to measure the PFNS in {sup 239}Pu(n,f) performed in 2008. Prompt fission neutron spectra in the neutron-induced fission of {sup 239}Pu have been measured for incident neutron energies from 1 to 200 MeV at the Los Alamos Neutron Science Center. Mean energies obtained from the spectra are discussed and compared to theoretical model calculation.

  19. Investigating Prompt Fission Neutron Emission from 235U(n,f) in the Resolved Resonance Region

    NASA Astrophysics Data System (ADS)

    Göök, Alf; Hambsch, Franz-Josef; Oberstedt, Stephan

    2016-03-01

    Investigations of prompt emission in fission is of importance in understanding the fission process in general and the sharing of excitation energy among the fission fragments in particular. Experimental activities at IRMM on prompt neutron emission from fission in response to OECD/NEA nuclear data requests is presented in this contribution. Main focus lies on currently on-going investigations of prompt neutron emission from the reaction 235U(n,f) in the region of the resolved resonances. For this reaction strong fluctuations of fission fragment mass distributions and mean total kinetic energy have been observed [Nucl. Phys. A 491, 56 (1989)] as a function of incident neutron energy in the resonance region. In addition fluctuations of prompt neutron multiplicities were also observed [Phys. Rev. C 13, 195 (1976)]. The goal of the present study is to verify the current knowledge of prompt neutron multiplicity fluctuations and to study correlations with fission fragment properties.

  20. Event-by-event study of prompt neutrons from 239Pu(n,f)

    SciTech Connect

    Vogt, R; Randrup, J; Pruet, J; Younes, W

    2009-07-23

    Employing a recently developed Monte-Carlo model, we study the fission of {sup 240}Pu induced by neutrons with energies from thermal to just below the threshold for second chance fission. Current measurements of the mean number of prompt neutrons emitted in fission, together with less accurate measurements of the neutron energy spectra, place remarkably fine constraints on predictions of microscopic calculations. In particular, the total excitation energy of the nascent fragments must be specified to within 1MeV to avoid disagreement with measurements of the mean neutron multiplicity. The combination of the Monte-Carlo fission model with a statistical likelihood analysis also presents a powerful tool for the evaluation of fission neutron data. Of particular importance is the fission spectrum, which plays a key role in determining reactor criticality. We show that our approach can be used to develop an estimate of the fission spectrum with uncertainties several times smaller than current experimental uncertainties for outgoing neutron energies of less than 2 MeV.

  1. Event-by-Event Study of Prompt Neutrons from 239Pu

    SciTech Connect

    Vogt, R; Randrup, J; Pruet, J; Younes, W

    2010-01-15

    Employing a recently developed Monte Carlo model, we study the fission of {sup 240}Pu induced by neutrons with energies from thermal to just below the threshold for second chance fission. Current measurements of the mean number of prompt neutrons emitted in fission, together with less accurate measurements of the neutron energy spectra, place remarkably fine constraints on predictions of microscopic calculations. In particular, the total excitation energy of the nascent fragments must be specified to within 1 MeV to avoid disagreement with measurements of the mean neutron multiplicity. The combination of the Monte Carlo fission model with a statistical likelihood analysis also presents a powerful tool for the evaluation of fission neutron data. Of particular importance is the fission spectrum, which plays a key role in determining reactor criticality. We show that our approach can be used to develop an estimate of the fission spectrum with uncertainties several times smaller than current experimental uncertainties for outgoing neutron energies of less than 2 MeV.

  2. Measurement of prompt fission neutron spectrum using a gamma tag double time-of-flight setup

    NASA Astrophysics Data System (ADS)

    Blain, Ezekiel

    Current uncertainties in the prompt fission neutron spectrum have a significant effect of up to 4% on keff for reactor criticality and safety calculations. Therefore, a method was developed at RPI to improve the accuracy of the measurement of the prompt fission neutron spectrum. This method involves using an array of BaF2 gamma detectors to tag that a fission event has occurred, and a double time-of-flight setup to obtain the prompt fission neutron spectrum as a function of incident neutron energy. The gamma tagging method improves upon conventional fission chambers by allowing for much larger sample sizes to be utilized while not suffering from effects of discriminator level on the shape of the prompt fission neutron spectrum. A coincidence requirement on an array of 4 BaF2 gamma detectors is used to determine the timing of the fission event. Furthermore, a method is under development for the use of thin plastic scintillators for measurement of the prompt fission neutron spectrum with low energies. Measurements with spontaneous fission of . {252} Cf show good agreement with previous datasets and current evaluations as well as providing accurate data down to 50 keV with the plastic scintillator detector. Preliminary incident neutron beam analysis was performed with 238U and shows good agreement with the current evaluations demonstrating the feasibility of the gamma tagging method for in beam prompt fission neutron spectrum measurements of various isotopes.

  3. Current Issues in Nuclear Data Evaluation Methodology: {sup 235}U Prompt Fission Neutron Spectra and Multiplicity for Thermal Neutrons

    SciTech Connect

    Trkov, A.; Capote, R.; Pronyaev, V.G.

    2015-01-15

    Issues in evaluation methodology of the prompt fission neutron spectra (PFNS) and neutron multiplicity for the thermal-neutron-induced fission of the {sup 235}U are discussed. The inconsistency between the experimental differential and integral data is addressed. By using differential data as ”shape data” good consistency was achieved between available sets of differential data. Integral dosimetry data have been used to define the PFNS slope at high outgoing neutron energies, where the quality of the differential data is poor. The inclusion into the fit of measured integral (spectrum-averaged) cross sections had a very small impact in the region where differential PFNS data are abundant and accurate, but removed the discrepancy with integral data at higher neutron emission energies. All experimental data are consistently fitted giving a PFNS average energy of 2.008 MeV. The impact on criticality prediction of the newly evaluated PFNS was tested. The highly enriched {sup 235}U solution assemblies with high leakage HEU-SOL-THERM-001 and HEU-SOL-THERM-009 benchmarks are the most sensitive to the PFNS. Criticality calculations for those solutions show a significant increase in reactivity if the average neutron energy of the fission neutrons is reduced from the ENDF/B-VI.5 value of 2.03 MeV. The proposed reduction of the PFNS average energy by 1.1% can be compensated by reducing the average number of neutrons per fission ν{sup ¯} at the thermal energy to the Gwin et al. measured value. The simple least-squares PFNS fit was confirmed by a more sophisticated combined fit of differential PFNS data for {sup 233,235}U, {sup 239}Pu and {sup 252}Cf nuclides with the generalised least-squares method using the GMA and GANDR codes.

  4. Current Issues in Nuclear Data Evaluation Methodology: 235U Prompt Fission Neutron Spectra and Multiplicity for Thermal Neutrons

    NASA Astrophysics Data System (ADS)

    Trkov, A.; Capote, R.; Pronyaev, V. G.

    2015-01-01

    Issues in evaluation methodology of the prompt fission neutron spectra (PFNS) and neutron multiplicity for the thermal-neutron-induced fission of the 235U are discussed. The inconsistency between the experimental differential and integral data is addressed. By using differential data as "shape data" good consistency was achieved between available sets of differential data. Integral dosimetry data have been used to define the PFNS slope at high outgoing neutron energies, where the quality of the differential data is poor. The inclusion into the fit of measured integral (spectrum-averaged) cross sections had a very small impact in the region where differential PFNS data are abundant and accurate, but removed the discrepancy with integral data at higher neutron emission energies. All experimental data are consistently fitted giving a PFNS average energy of 2.008 MeV. The impact on criticality prediction of the newly evaluated PFNS was tested. The highly enriched 235U solution assemblies with high leakage HEU-SOL-THERM-001 and HEU-SOL-THERM-009 benchmarks are the most sensitive to the PFNS. Criticality calculations for those solutions show a significant increase in reactivity if the average neutron energy of the fission neutrons is reduced from the ENDF/B-VI.5 value of 2.03 MeV. The proposed reduction of the PFNS average energy by 1.1% can be compensated by reducing the average number of neutrons per fission νbar at the thermal energy to the Gwin et al. measured value. The simple least-squares PFNS fit was confirmed by a more sophisticated combined fit of differential PFNS data for 233,235U, 239Pu and 252Cf nuclides with the generalised least-squares method using the GMA and GANDR codes.

  5. Prompt gamma and neutron detection in BNCT utilizing a CdTe detector.

    PubMed

    Winkler, Alexander; Koivunoro, Hanna; Reijonen, Vappu; Auterinen, Iiro; Savolainen, Sauli

    2015-12-01

    In this work, a novel sensor technology based on CdTe detectors was tested for prompt gamma and neutron detection using boronated targets in (epi)thermal neutron beam at FiR1 research reactor in Espoo, Finland. Dedicated neutron filter structures were omitted to enable simultaneous measurement of both gamma and neutron radiation at low reactor power (2.5 kW). Spectra were collected and analyzed in four different setups in order to study the feasibility of the detector to measure 478 keV prompt gamma photons released from the neutron capture reaction of boron-10. The detector proved to have the required sensitivity to detect and separate the signals from both boron neutron and cadmium neutron capture reactions, which makes it a promising candidate for monitoring the spatial and temporal development of in vivo boron distribution in boron neutron capture therapy. PMID:26249745

  6. Prompt Gamma-Ray Neutron Activation Analysis (PGNAA) for Elemental Analysis

    SciTech Connect

    Robin P. Gardner

    2006-04-11

    This research project was to improve the prompt gamma-ray neutron activation analysis (PGNAA) measurement approach for bulk analysis, oil well logging, and small sample thermal enutron bean applications.

  7. Method for measuring prompt γ-rays generated by D-T neutrons bombarding a depleted uranium spherical shell

    NASA Astrophysics Data System (ADS)

    Qin, Jian-Guo; Lai, Cai-Feng; Jiang, Li; Liu, Rong Zhang, Xin-Wei; Ye, Bang-Jiao; Zhu, Tong-Hua

    2016-01-01

    The prompt γ-ray spectrum from depleted uranium (DU) spherical shells induced by 14 MeV D-T neutrons is measured. Monte Carlo (MC) simulation gives the largest prompt γ flux with the optimal thickness of the DU spherical shells 3-5 cm and the optimal frequency of neutron pulse 1 MHz. The method of time of flight and pulse shape coincidence with energy (DC-TOF) is proposed, and the subtraction of the background γ-rays discussed in detail. The electron recoil spectrum and time spectrum of the prompt γ-rays are obtained based on a 2″×2″ BC501A liquid scintillator detector. The energy spectrum and time spectrum of prompt γ-rays are obtained based on an iterative unfolding method that can remove the influence of γ-rays response matrix and pulsed neutron shape. The measured time spectrum and the calculated results are roughly consistent with each other. Experimental prompt γ-ray spectrum in the 0.4-3 MeV energy region agrees well with MC simulation based on the ENDF/BVI.5 library, and the discrepancies for the integral quantities of γ-rays of energy 0.4-1 MeV and 1-3 MeV are 9.2% and 1.1%, respectively. Supported by National Special Magnetic Confinement Fusion Energy Research, China (2015GB108001) and National Natural Science Foundation of China (91226104)

  8. Development Of A Digital Technique For The Determination Of Fission Fragments And Emitted Prompt Neutron Characteristics

    NASA Astrophysics Data System (ADS)

    Varapai, N.; Hambsch, F.-J.; Oberstedt, S.; Serot, O.; Barreau, G.; Kornilov, N.; Zeinalov, Sh.

    2005-11-01

    The present work demonstrates the application of the digital technique for nuclear measurements. This method has been implemented for measurements of promptly emitted fission neutrons in coincidence with fission fragments from 252Cf(sf). A double Frisch-grid ionization chamber is used as fission fragment detector. The promptly emitted neutrons are detected by a NE213 liquid scintillation detector. The experimental set-up is installed at the Institute for Reference Materials and Measurements. Preliminary results are presented.

  9. Measurements of prompt radiation induced conductivity in Teflon (PTFE).

    SciTech Connect

    Hartman, E. Frederick; Zarick, Thomas Andrew; Sheridan, Timothy J.; Preston, E.

    2013-05-01

    We performed measurements of the prompt radiation induced conductivity (RIC) in thin samples of Teflon (PTFE) at the Little Mountain Medusa LINAC facility in Ogden, UT. Three mil (76.2 microns) samples were irradiated with a 0.5 %CE%BCs pulse of 20 MeV electrons, yielding dose rates of 1E9 to 1E11 rad/s. We applied variable potentials up to 2 kV across the samples and measured the prompt conduction current. Details of the experimental apparatus and analysis are reported in this report on prompt RIC in Teflon.

  10. Measurements of prompt radiation induced conductivity of Kapton.

    SciTech Connect

    Preston, Eric F.; Zarick, Thomas Andrew; Sheridan, Timothy J.; Hartman, E. Frederick; Stringer, Thomas Arthur

    2010-10-01

    We performed measurements of the prompt radiation induced conductivity in thin samples of Kapton (polyimide) at the Little Mountain Medusa LINAC facility in Ogden, UT. Three mil samples were irradiated with a 0.5 {mu}s pulse of 20 MeV electrons, yielding dose rates of 1E9 to 1E10 rad/s. We applied variable potentials up to 2 kV across the samples and measured the prompt conduction current. Analysis rendered prompt conductivity coefficients between 6E-17 and 2E-16 mhos/m per rad/s, depending on the dose rate and the pulse width.

  11. Uranium and Plutonium Average Prompt-fission Neutron Energy Spectra (PFNS) from the Analysis of NTS NUEX Data

    NASA Astrophysics Data System (ADS)

    Lestone, J. P.; Shores, E. F.

    2014-05-01

    In neutron experiments (NUEX) conducted at the Nevada Test Site (NTS) by Los Alamos National Laboratory, the time-of-flight of fission-neutrons emitted from nuclear tests were observed by measuring the current generated by the collection of protons scattered from a thin CH2 foil many meters from the nuclear device into a Faraday cup. The time dependence of the Faraday cup current is a measure of the energy spectrum of the neutrons that leak from the device. With good device models and accurate neutron-transport codes, the leakage spectra can be converted into prompt fast-neutron-induced fission-neutron energy spectra. This has been done for two events containing plutonium, and for an earlier event containing uranium. The prompt-fission neutron spectra have been inferred for 1.5-MeV 239Pu(n,f) and 235U(n,f) reactions for outgoing neutron energies from 1.5 to ∼10.5 MeV, in 1-MeV steps. These spectra are in good agreement with the Los Alamos fission model.

  12. The Prompt Gamma Neutron Activation Analysis Facility at ICN-Pitesti

    SciTech Connect

    Barbos, D.; Paunoiu, C.; Mladin, M.; Cosma, C.

    2008-08-14

    PGNAA is a very widely applicable technique for determining the presence and amount of many elements simultaneously in samples ranging in size from micrograms to many grams. PGNAA is characterized by its capability for nondestructive multi-elemental analysis and its ability to analyse elements that cannot be determined by INAA. By means of this PGNAA method we are able to increase the performance of INAA method. A facility has been developed at Institute for Nuclear Research-Pitesti so that the unique features of prompt gamma-ray neutron activation analysis can be used to measure trace and major elements in samples. The facility is linked at the radial neutron beam tube at ACPR-TRIGA reactor. During the PGNAA-facility is in use the ACPR reactor will be operated in steady-state mode at 250 KW maximum power. The facility consists of a radial beam-port, external sample position with shielding, and induced prompt gamma-ray counting system.Thermal neutron flux with energy lower than cadmium cut-off at the sample position was measured using thin gold foil is: {phi}{sub scd} = 1.10{sup 6} n/cm{sup 2}/s with a cadmium ratio of:80.The gamma-ray detection system consist of an HpGe detector of 16% efficiency (detector model GC1518) with 1.85 keV resolution capability. The HpGe is mounted with its axis at 90 deg. with respect to the incident neutron beam at distance about 200mm from the sample position. To establish the performance capabilities of the facility, irradiation of pure element or sample compound standards were performed to identify the gama-ray energies from each element and their count rates.

  13. Prompt gamma-ray analysis using cold and thermal guided neutron beams at JAERI.

    PubMed

    Yonezawa, C

    1999-01-01

    A highly sensitive neutron-induced prompt gamma-ray analysis (PGA) system, usable at both cold and thermal neutron beam guides of JRR-3M, has been constructed. The system was designed to achieve the lowest gamma-ray background by using lithium fluoride tiles as neutron shielding, by placing the samples in a He atmosphere and by using a Ge-bismuth germanate detector system for Compton suppression. The gamma-ray spectrometer can acquire three modes of spectra simultaneously: single, Compton suppression, and pair modes. Because of the low-energy guided neutron beams and the low-background system, analytical sensitivities and detection limits better than those in usual PGA systems have been achieved. Boron and multielemental determination by a comparative standardization have been investigated, and accuracy, precision, and detection limits for the elements in various materials were evaluated. The system has been applied to the determination of B and multielements in samples of various fields such as medical, environmental, and geological sciences. PMID:10676516

  14. Non destructive multi elemental analysis using prompt gamma neutron activation analysis techniques: Preliminary results for concrete sample

    SciTech Connect

    Dahing, Lahasen Normanshah; Yahya, Redzuan; Yahya, Roslan; Hassan, Hearie

    2014-09-03

    In this study, principle of prompt gamma neutron activation analysis has been used as a technique to determine the elements in the sample. The system consists of collimated isotopic neutron source, Cf-252 with HPGe detector and Multichannel Analysis (MCA). Concrete with size of 10×10×10 cm{sup 3} and 15×15×15 cm{sup 3} were analysed as sample. When neutrons enter and interact with elements in the concrete, the neutron capture reaction will occur and produce characteristic prompt gamma ray of the elements. The preliminary result of this study demonstrate the major element in the concrete was determined such as Si, Mg, Ca, Al, Fe and H as well as others element, such as Cl by analysis the gamma ray lines respectively. The results obtained were compared with NAA and XRF techniques as a part of reference and validation. The potential and the capability of neutron induced prompt gamma as tool for multi elemental analysis qualitatively to identify the elements present in the concrete sample discussed.

  15. Stability evaluation and correction of a pulsed neutron generator prompt gamma activation analysis system

    Technology Transfer Automated Retrieval System (TEKTRAN)

    Source output stability is important for accurate measurement in prompt gamma neutron activation. This is especially true when measuring low-concentration elements such as in vivo nitrogen (~2.5% of body weight). We evaluated the stability of the compact DT neutron generator within an in vivo nitrog...

  16. Prompt neutron decay for an unreflected and unmoderated uranium (HEU) metal sphere

    SciTech Connect

    Mihalczo, J.T.

    1996-08-01

    Prompt neutron decay constants were measured for a delayed critical, unmoderated and unreflected U metal sphere at the Oak Ridge Critical Experiments Facility. Prompt neutron decay constant was 1.1095{+-}0.0013 {mu}s{sup -1}. This can be used to verify calculational methods, both deterministic and Monte Carlo neutron transport methods. This value is in agreement with the value from GODIVA I data corrected for effects of support structure (1.10{+-}0.01 {mu}s{sup -1}) but has a much smaller error as a result of the large number (167) of the measurements here and the high degree of sphericity of the sphere.

  17. Utilization of Actively-induced, Prompt Radiation Emission for Nonproliferation Applications

    SciTech Connect

    F. W. Blackburn; J. L. Jones; C. E. Moss; J. T. Mihalzco; A. W. Hunt; F. Harmon

    2006-08-01

    The pulsed Photonuclear Assessment (PPA) technique, which has demonstrated the ability to detect shielded nuclear material, is based on utilizing delayed neutrons and photons between accelerator pulses. While most active interrogation systems have focused on delayed neutron and gamma-ray signatures, the current requirements of various agencies necessitate bringing faster detection and acquisition capabilities to field inspection applications. This push for decreased interrogation times, increased sensitivity and mitigation of false positives requires that detection systems take advantage of all available information. Collaborative research between Idaho National Lab (INL), Idaho State University’s Idaho Accelerator Center (IAC), Los Alamos National Laboratory (LANL), and Oak Ridge National Laboratory (ORNL), has focused on exploiting actively-induced, prompt radiation signatures from nuclear material within a pulsed photonuclear environment. To date, these prompt emissions have not been effectively exploited due to difficulties in detection and signal processing inherent in the prompt regime as well as an overall poor understanding of the magnitude and yields of these emissions. Exploitation of prompt radiation (defined as during an accelerator pulse/(photo) fission event and/or immediately after (< l ms)) has the potential to dramatically reduce interrogation times since the yields are more than two orders of magnitude greater than delayed emissions. Recent preliminary experiments conducted at the IAC suggest that it is indeed possible to extract prompt neutron information within a pulsed photon environment. Successful exploitation of prompt emissions is critical for the development of an improved robust, high-throughput, low target dose inspection system for detection of shielded nuclear materials.

  18. Determination of boron in materials by cold neutron prompt gamma-ray activation analysis.

    PubMed

    Paul, Rick L

    2005-01-01

    An instrument for cold neutron prompt gamma-ray activation analysis (PGAA), located at the NIST Center for Neutron Research (NCNR), has proven useful for the measurement of boron in a variety of materials. Neutrons, moderated by passage through liquid hydrogen at 20 K, pass through a (58)Ni coated guide to the PGAA station in the cold neutron guide hall of the NCNR. The thermal equivalent neutron fluence rate at the sample position is 9 x 10(8) cm(-2) s(-1). Prompt gamma rays are measured by a cadmium- and lead-shielded high-purity germanium detector. The instrument has been used to measure boron mass fractions in minerals, in NIST SRM 2175 (Refractory Alloy MP-35-N) for certification of boron, and most recently in semiconductor-grade silicon. The limit of detection for boron in many materials is <10 ng g(-1). PMID:15614360

  19. Utilization of recycled neutron source to teach prompt gamma analysis activation-PGNA

    NASA Astrophysics Data System (ADS)

    Delgado-Correal, Camilo; Munera, Hector

    2008-03-01

    Neutron activation analysis based on prompt gamma ray emission has significantly developed during the past twenty years. The technique is particularly suited for the identification of low atomic number elements, as nitrogen that is a main component of drugs and explosives. Identification of these substances is important in the context of humanitarian demining, and in the control of illicit traffic of drugs and explosives. As a good example of recycling of radioactive sources, a ^241Am-Be neutron source emitting 10^7neutron/s, that was not longer in use for other purposes at Ingeominas, was used to build a neutron irradiator that can be used to teach prompt gamma ray analysis, and other nuclear techniques. We irradiated individual samples, each about 4 gram, of three different elements: nitrogen in urea, silicon in milled rock, and cadmium in cadmium oxide. The prompt gamma rays emitted in the nuclear reactions ^112Cd (neutron,gamma) ^113Cd, ^28Si (neutron,gamma) ^29Si and ^14N (neutron,gamma) ^15N were identified using a well-type NaI (Tl) detector, connected to a multi-channel analyzer.

  20. Measurements of prompt radiation induced conductivity of alumina and sapphire.

    SciTech Connect

    Hartman, E. Frederick; Zarick, Thomas Andrew; Sheridan, Timothy J.; Preston, Eric F.

    2011-04-01

    We performed measurements of the prompt radiation induced conductivity in thin samples of Alumina and Sapphire at the Little Mountain Medusa LINAC facility in Ogden, UT. Five mil thick samples were irradiated with pulses of 20 MeV electrons, yielding dose rates of 1E7 to 1E9 rad/s. We applied variable potentials up to 1 kV across the samples and measured the prompt conduction current. Analysis rendered prompt conductivity coefficients between 1E10 and 1E9 mho/m/(rad/s), depending on the dose rate and the pulse width for Alumina and 1E7 to 6E7 mho/m/(rad/s) for Sapphire.

  1. The LICORNE Neutron Source and Measurements of Prompt γ-rays Emitted in Fission

    NASA Astrophysics Data System (ADS)

    Wilson, J. N.; Lebois, M.; Halipre, P.; Oberstedt, S.; Oberstedt, A.

    The emission of prompt gamma rays is one of the least measured and least well-understood parts of the fission process. Knowledge of prompt fission gamma spectra, mean energies and multiplicities are important for reactor gamma heating and hence linked to reactor safety. At the IPN Orsay we have developed a unique, directional, fast neutron source called LICORNE, intended initially to facilitate prompt fission gamma measurements. The ability of the IPN Orsay tandem accelerator to produce intense beams of 7Li is exploited to produce quasi mono-energetic neutrons between 0.5 - 4 MeV using the p(7Li, 7Be)n inverse reaction. The available fluxes of up to 7×107 neutrons/second/steradian are comparable to existing installations, but with two added advantages: (i) The kinematic focusing produces a natural neutron beam collimation which allows placement of gamma detectors adjacent to the irradiated sample unimpeded by source neutrons. (ii) The background of scattered neutrons in the experimental hall is drastically reduced. The dedicated neutron converter was commissioned in June 2013

  2. Angular correlations in emission of prescission neutrons from {sup 235}U fission induced by slow polarized neutrons

    SciTech Connect

    Danilyan, G. V.; Wilpert, T.; Granz, P.; Krakhotin, V. A.; Mezei, F.; Novitsky, V. V.; Pavlov, V. S.; Russina, M. V.; Shatalov, P. B.

    2008-12-15

    A new approach to searching for and studying scission neutrons, which is based on the analysis of specific angular correlations in nuclear fission induced by polarized neutrons, is described and used to evaluate the fraction of scission neutrons in the total number of prompt neutrons of {sup 235}U fission emitted perpendicularly to the fission axis.

  3. Use of borated polyethylene to improve low energy response of a prompt gamma based neutron dosimeter

    NASA Astrophysics Data System (ADS)

    Priyada, P.; Ashwini, U.; Sarkar, P. K.

    2016-05-01

    The feasibility of using a combined sample of borated polyethylene and normal polyethylene to estimate neutron ambient dose equivalent from measured prompt gamma emissions is investigated theoretically to demonstrate improvements in low energy neutron dose response compared to only polyethylene. Monte Carlo simulations have been carried out using the FLUKA code to calculate the response of boron, hydrogen and carbon prompt gamma emissions to mono energetic neutrons. The weighted least square method is employed to arrive at the best linear combination of these responses that approximates the ICRP fluence to dose conversion coefficients well in the energy range of 10-8 MeV to 14 MeV. The configuration of the combined system is optimized through FLUKA simulations. The proposed method is validated theoretically with five different workplace neutron spectra with satisfactory outcome.

  4. Investigation of the prompt-neutron spectrum for spontaneously-fissioning /sup 252/Cf

    SciTech Connect

    Poenitz, W.P.; Tamura, T.

    1982-01-01

    The prompt-fission-neutron spectrum of /sup 252/Cf was investigated. The spectrum was measured with Black Neutron Detectors which have a well known efficiency. Considerations of various issues in such measurements lead to an experiment in which a time-calibration pulser, a random pulser, the neutron detector time-of-flight spectrum, the pulse-shape-discriminator gamma time-of-flight spectrum, and the detector-response spectra were simultaneously recorded for the prompt-fission neutrons, transmission through carbon, and shadowbars in a total-cross-section-type measurement. Corrections and associated uncertainties were applied for a large variety of effects which may have been overlooked in many of the previously reported measurements. Preliminary results indicate deviations from a Maxwellian shape toward a Watt-spectrum shape. Agreement is good with the shape differences relative to a Maxwellian from the recent theoretical calculation by Madland and Nix, however, a lower average energy was found.

  5. The 235U Prompt Fission Neutron Spectrum in the BR1 Reactor at SCK•CEN

    NASA Astrophysics Data System (ADS)

    Wagemans, Jan; Malambu, Edouard; Borms, Luc; Fiorito, Luca

    2016-02-01

    The BR1 research reactor at SCK•CEN has a spherical cavity in the graphite above the reactor core. In this cavity an accurately characterised Maxwellian thermal neutron field is present. Different converters can be loaded in the cavity in order to obtain other types of neutron (and gamma) irradiation fields. Inside the so-called MARK III converter a fast 235U(n,f) prompt fission neutron field can be obtained. With the support of MCNP calculations, irradiations in MARK III can be directly related to the pure 235U(n,f) prompt fission neutron spectrum. For this purpose MARK III spectrum averaged cross sections for the most relevant fluence dosimetry reactions have been determined. A calibration factor for absolute measurements has been determined applying activation dosimetry following ISO/IEC 17025 standards.

  6. A compact neutron beam generator system designed for prompt gamma nuclear activation analysis.

    PubMed

    Ghassoun, J; Mostacci, D

    2011-08-01

    In this work a compact system was designed for bulk sample analysis using the technique of PGNAA. The system consists of (252)Cf fission neutron source, a moderator/reflector/filter assembly, and a suitable enclosure to delimit the resulting neutron beam. The moderator/reflector/filter arrangement has been optimised to maximise the thermal neutron component useful for samples analysis with a suitably low level of beam contamination. The neutron beam delivered by this compact system is used to irradiate the sample and the prompt gamma rays produced by neutron reactions within the sample elements are detected by appropriate gamma rays detector. Neutron and gamma rays transport calculations have been performed using the Monte Carlo N-Particle transport code (MCNP5). PMID:21129990

  7. Monte Carlo Predictions of Prompt Fission Neutrons and Photons: a Code Comparison

    NASA Astrophysics Data System (ADS)

    Talou, P.; Kawano, T.; Stetcu, I.; Vogt, R.; Randrup, J.

    2014-04-01

    This paper reports on initial comparisons between the LANL CGMF and LBNL/LLNL FREYA codes, which both aim at computing prompt fission neutrons and gammas. While the methodologies used in both codes are somewhat similar, the detailed implementations and physical assumptions are different. We are investigating how some of these differences impact predictions.

  8. Development of a new deuterium-deuterium (D-D) neutron generator for prompt gamma-ray neutron activation analysis.

    PubMed

    Bergaoui, K; Reguigui, N; Gary, C K; Brown, C; Cremer, J T; Vainionpaa, J H; Piestrup, M A

    2014-12-01

    A new deuterium-deuterium (D-D) neutron generator has been developed by Adelphi Technology for prompt gamma neutron activation analysis (PGNAA), neutron activation analysis (NAA), and fast neutron radiography. The generator makes an excellent fast, intermediate, and thermal neutron source for laboratories and industrial applications that require the safe production of neutrons, a small footprint, low cost, and small regulatory burden. The generator has three major components: a Radio Frequency Induction Ion Source, a Secondary Electron Shroud, and a Diode Accelerator Structure and Target. Monoenergetic neutrons (2.5MeV) are produced with a yield of 10(10)n/s using 25-50mA of deuterium ion beam current and 125kV of acceleration voltage. The present study characterizes the performance of the neutron generator with respect to neutron yield, neutron production efficiency, and the ionic current as a function of the acceleration voltage at various RF powers. In addition the Monte Carlo N-Particle Transport (MCNP) simulation code was used to optimize the setup with respect to thermal flux and radiation protection. PMID:25305524

  9. Using anisotropies in prompt fission neutron coincidences to assess the neutron multiplication of highly multiplying subcritical plutonium assemblies

    NASA Astrophysics Data System (ADS)

    Mueller, J. M.; Mattingly, J.

    2016-07-01

    There is a significant and well-known anisotropy between the prompt neutrons emitted from a single fission event; these neutrons are most likely to be observed at angles near 0° or 180° relative to each other. However, the propagation of this anisotropy through different generations of a fission chain reaction has not been previously studied. We have measured this anisotropy in neutron-neutron coincidences from a subcritical highly-multiplying assembly of plutonium metal. The assembly was a 4.5 kg α-phase plutonium metal sphere composed of 94% 239Pu and 6% 240Pu by mass. Data were collected using two EJ-309 liquid scintillators and two EJ-299 plastic scintillators. The angular distribution of neutron-neutron coincidences was measured at 90° and 180° and found to be largely isotropic. Simulations were performed using MCNPX-PoliMi of similar plutonium metal spheres of varying sizes and a correlation between the neutron multiplication of the assembly and the anisotropy of neutron-neutron coincidences was observed. In principle, this correlation could be used to assess the neutron multiplication of an unknown assembly.

  10. Prompt fission neutron spectra of n+235U above the (n,nf) fission threshold

    NASA Astrophysics Data System (ADS)

    Shu, Neng-Chuan; Jia, Min; Chen, Yong-Jing; Liu, Ting-Jin

    2015-05-01

    Calculations of prompt fission neutron spectra (PFNS) from the 235U(n, f) reaction were performed with a semi-empirical method for En = 7.0 and 14.7 MeV neutron energies. The total PFNS were obtained as a superposition of (n,xnf) pre-fission neutron spectra and post-fission spectra of neutrons which were evaporated from fission fragments, and these two kinds of spectra were taken as an expression of the evaporation spectrum. The contributions of (n,xnf) fission neutron spectra on the calculated PFNS were discussed. The results show that emission of one or two neutrons in the (n,nf) or (n,2nf) reactions influences the PFNS shape, and the neutron spectra of the (n,xnf) fission-channel are soft compared with the neutron spectra of the (n,f) fission channel. In addition, analysis of the multiple-chance fission component showed that second-chance fission dominates the PFNS with an incident neutron energy of 14.7 MeV whereas first-chance fission dominates the 7 MeV case. Supported by National Natural Science Foundation of China (11205246, 91126010, U1230127, 91226102), IAEA CRP (15905), and Defense Industrial Technology Development Program (B0120110034)

  11. Spin distribution in neutron induced preequilibrium reactions

    SciTech Connect

    Dashdorj, D; Kawano, T; Chadwick, M; Devlin, M; Fotiades, N; Nelson, R O; Mitchell, G E; Garrett, P E; Agvaanluvsan, U; Becker, J A; Bernstein, L A; Macri, R; Younes, W

    2005-10-04

    The preequilibrium reaction mechanism makes an important contribution to neutron-induced reactions above E{sub n} {approx} 10 MeV. The preequilibrium process has been studied exclusively via the characteristic high energy neutrons produced at bombarding energies greater than 10 MeV. They are expanding the study of the preequilibrium reaction mechanism through {gamma}-ray spectroscopy. Cross-section measurements were made of prompt {gamma}-ray production as a function of incident neutron energy (E{sub n} = 1 to 250 MeV) on a {sup 48}Ti sample. Energetic neutrons were delivered by the Los Alamos National Laboratory spallation neutron source located at the Los Alamos Neutron Science Center facility. The prompt-reaction {gamma} rays were detected with the large-scale Compton-suppressed Germanium Array for Neutron Induced Excitations (GEANIE). Neutron energies were determined by the time-of-flight technique. The {gamma}-ray excitation functions were converted to partial {gamma}-ray cross sections taking into account the dead-time correction, target thickness, detector efficiency and neutron flux (monitored with an in-line fission chamber). Residual state population was predicted using the GNASH reaction code, enhanced for preequilibrium. The preequilibrium reaction spin distribution was calculated using the quantum mechanical theory of Feshback, Kerman, and Koonin (FKK). The multistep direct part of the FKK theory was calculated for a one-step process. The FKK preequilibrium spin distribution was incorporated into the GNASH calculations and the {gamma}-ray production cross sections were calculated and compared with experimental data. The difference in the partial {gamma}-ray cross sections using spin distributions with and without preequilibrium effects is significant.

  12. Database of prompt gamma rays from slow neutron capture forelemental analysis

    SciTech Connect

    Firestone, R.B.; Choi, H.D.; Lindstrom, R.M.; Molnar, G.L.; Mughabghab, S.F.; Paviotti-Corcuera, R.; Revay, Zs; Trkov, A.; Zhou,C.M.; Zerkin, V.

    2004-12-31

    The increasing importance of Prompt Gamma-ray ActivationAnalysis (PGAA) in a broad range of applications is evident, and has beenemphasized at many meetings related to this topic (e.g., TechnicalConsultants' Meeting, Use of neutron beams for low- andmedium-fluxresearch reactors: radiography and materialscharacterizations, IAEA Vienna, 4-7 May 1993, IAEA-TECDOC-837, 1993).Furthermore, an Advisory Group Meeting (AGM) for the Coordination of theNuclear Structure and Decay Data Evaluators Network has stated that thereis a need for a complete and consistent library of cold- and thermalneutron capture gammaray and cross-section data (AGM held at Budapest,14-18 October 1996, INDC(NDS)-363); this AGM also recommended theorganization of an IAEA CRP on the subject. The International NuclearData Committee (INDC) is the primary advisory body to the IAEA NuclearData Section on their nuclear data programmes. At a biennial meeting in1997, the INDC strongly recommended that the Nuclear Data Section supportnew measurements andupdate the database on Neutron-induced PromptGamma-ray Activation Analysis (21st INDC meeting, INDC/P(97)-20). As aconsequence of the various recommendations, a CRP on "Development of aDatabase for Prompt Gamma-ray Neutron Activation Analysis (PGAA)" wasinitiated in 1999. Prior to this project, several consultants had definedthe scope, objectives and tasks, as approved subsequently by the IAEA.Each CRP participant assumed responsibility for the execution of specifictasks. The results of their and other research work were discussed andapproved by the participants in research co-ordination meetings (seeSummary reports: INDC(NDS)-411, 2000; INDC(NDS)-424, 2001; andINDC(NDS)-443, 200). PGAA is a non-destructive radioanalytical method,capable of rapid or simultaneous "in-situ" multi-element analyses acrossthe entire Periodic Table, from hydrogen to uranium. However, inaccurateand incomplete data were a significant hindrance in the qualitative andquantitative

  13. A method to measure prompt fission neutron spectrum using gamma multiplicity tagging

    NASA Astrophysics Data System (ADS)

    Blain, E.; Daskalakis, A.; Block, R. C.; Barry, D.; Danon, Y.

    2016-01-01

    In order to improve on current prompt fission neutron spectrum measurements, a gamma multiplicity tagging method was developed at the Rensselaer Polytechnic Institute Gearttner Linear Accelerator Center. This method involves using a coincidence requirement on an array of BaF2 gamma detectors to determine the timing of a fission event. This allows for much larger fission samples to be used due to the higher penetrability of gammas compared to fission fragments. Additionally, since the method relies on gammas as opposed to fission fragments, the effects of the low level discriminator, used in fission chambers to eliminate alpha events, are not seen. A 252Cf fission chamber was constructed in order to determine the viability of this method as well as the efficiency when compared to a fission chamber. The implemented multiple gamma tagging method was found to accurately reproduce the prompt fission neutron spectrum for the spontaneous fission of 252Cf and to detect 30% of fission events.

  14. Estimation of Covariances on Prompt Fission Neutron Spectra and Impact of the PFNS Model on the Vessel Fluence

    NASA Astrophysics Data System (ADS)

    Berge, Léonie; Litaize, Olivier; Serot, Olivier; Archier, Pascal; De Saint Jean, Cyrille; Pénéliau, Yannick; Regnier, David

    2016-02-01

    As the need for precise handling of nuclear data covariances grows ever stronger, no information about covariances of prompt fission neutron spectra (PFNS) are available in the evaluated library JEFF-3.2, although present in ENDF/B-VII.1 and JENDL-4.0 libraries for the main fissile isotopes. The aim of this work is to provide an estimation of covariance matrices related to PFNS, in the frame of some commonly used models for the evaluated files, such as the Maxwellian spectrum, the Watt spectrum, or the Madland-Nix spectrum. The evaluation of PFNS through these models involves an adjustment of model parameters to available experimental data, and the calculation of the spectrum variance-covariance matrix arising from experimental uncertainties. We present the results for thermal neutron induced fission of 235U. The systematic experimental uncertainties are propagated via the marginalization technique available in the CONRAD code. They are of great influence on the final covariance matrix, and therefore, on the spectrum uncertainty band width. In addition to this covariance estimation work, we have also investigated the importance on a reactor calculation of the fission spectrum model choice. A study of the vessel fluence depending on the PFNS model is presented. This is done through the propagation of neutrons emitted from a fission source in a simplified PWR using the TRIPOLI-4® code. This last study includes thermal fission spectra from the FIFRELIN Monte-Carlo code dedicated to the simulation of prompt particles emission during fission.

  15. Prompt neutron multiplicity in correlation with fragments from spontaneous fission of 252Cf

    NASA Astrophysics Data System (ADS)

    Göök, A.; Hambsch, F.-J.; Vidali, M.

    2014-12-01

    The spontaneous fission of 252Cf serves as an excellent benchmark of prompt emission in fission since experimental data can be obtained without the need of an incident beam. With the purpose of providing experimental data on the prompt fission neutron properties in correlation with fission-fragment characteristics, an experiment on 252Cf(SF) has been performed. In addition, the experiment serves as a benchmark of setup and analysis procedures for measurements of fluctuations in the prompt-neutron properties as a function of incident neutron energy in fission of the major actinides 235U and 239Pu. The experiment employs a twin Frisch grid ionization chamber as fission-fragment detector while neutrons were counted by using a liquid scintillator placed along the symmetry axis of the ionization chamber. Average neutron multiplicity has been obtained as a function of fission-fragment mass and total kinetic energy (TKE). The average multiplicity as a function of mass agrees well with available data in the literature in the mass range from 80 to 170 u. The existence of additional sawtooth structures in the far asymmetric mass region could not be confirmed, although the statistical accuracy of the present experiment is as good as the previous study where such structures have been reported [Nucl. Phys. A 490, 307 (1988)., 10.1016/0375-9474(88)90508-8]. The available data in the literature on the TKE dependence of the multiplicity show strong deviations. Therefore, effort was focused on investigating experimental factors in low-efficiency neutron-counting experiments that may lead to faulty determination of this dependence. Taking these factors into account, a result that agrees well with data from high-efficiency neutron-counting experiments is obtained. The experimental arrangement allows determination of the angle between the detected neutron and the fission axis, which permits the neutron properties to be transformed into the fission-fragment rest frame. Fission neutron

  16. A position-sensitive twin ionization chamber for fission fragment and prompt neutron correlation experiments

    NASA Astrophysics Data System (ADS)

    Göök, A.; Geerts, W.; Hambsch, F.-J.; Oberstedt, S.; Vidali, M.; Zeynalov, Sh.

    2016-09-01

    A twin position-sensitive Frisch grid ionization chamber, intended as a fission fragment detector in experiments to study prompt fission neutron correlations with fission fragment properties, is presented. Fission fragment mass and energies are determined by means of the double kinetic energy technique, based on conservation of mass and linear momentum. The position sensitivity is achieved by replacing each anode plate in the standard twin ionization chamber by a wire plane and a strip anode, both readout by means of resistive charge division. This provides information about the fission axis orientation, which is necessary to reconstruct the neutron emission process in the fully accelerated fragment rest-frame. The energy resolution compared to the standard twin ionization chamber is found not to be affected by the modification. The angular resolution of the detector relative to an arbitrarily oriented axis is better than 7° FWHM. Results on prompt fission neutron angular distributions in 235U(n,f) obtained with the detector in combination with an array of neutron scintillation detectors is presented as a proof of principle.

  17. Transitions, cross sections and neutron binding energy in 186Re by Prompt Gamma Activation Analysis

    NASA Astrophysics Data System (ADS)

    Lerch, A. G.; Hurst, A. M.; Firestone, R. B.; Revay, Zs.; Szentmiklosi, L.; McHale, S. R.; McClory, J. W.; Detwiler, B.; Carroll, J. J.

    2014-03-01

    The nuclide 186Re possesses an isomer with 200,000 year half-life while its ground state has a half-life of 3.718 days. It is also odd-odd and well-deformed nucleus, so should exhibit a variety of other interesting nuclear-structure phenomena. However, the available nuclear data is rather sparse; for example, the energy of the isomer is only known to within + 7 keV and, with the exception of the J?=1- ground state, every proposed level is tentative in the ENSDF. Previously, Prompt Gamma Activation Analysis (PGAA) was utilized to study natRe with 186,188Re being produced via thermal neutron capture. Recently, an enriched 185Re target was irradiated by thermal neutrons at the Budapest Research Reactor to build on those results. Prompt (primary and secondary) and delayed gamma-ray transitions were measured with a large-volume, Compton-suppressed HPGe detector. Absolute cross sections for each gamma transition were deduced and corrected for self attenuation within the sample. Fifty-two primary gamma-ray transitions were newly identified and used to determine a revised value of the neutron binding energy. DICEBOX was used to simulate the decay scheme and the total radiative thermal neutron capture cross section was found to be 97+/-3 b Supported by DTRA (Detwiler) through HDTRA1-08-1-0014.

  18. Determining plutonium mass in spent fuel using Cf-252 interrogation with prompt neutron detection

    SciTech Connect

    Hu, Jianwei; Tobin, Stephen J; Menlove, Howard O; Croft, Stephen

    2010-01-01

    {sup 252}Cf Interrogation with Prompt Neutron (CIPN) detection is proposed as one of 14 NDA techniques to determine Pu mass in spent fuel assemblies (FAs). CIPN is a low-cost and portable instrument, and it looks like a modified fork detector combined with an active interrogation source. Fission chamber (FC) is chosen as neutron detector because of its insensitivity to {gamma} radiation. The CIPN assay is comprised of two measurements, a background count and an active count, without and with the {sup 252}Cf source next to the fuel respectively. The net signal above background is primarily due to the multiplication of Cf source neutrons caused by the fissile content. The capability of CIPN to detect diversion and to determine fissile content was quantified using MCNPX simulations. New schemes were proposed (such as burnup and cooling time correction, etc.) and the results show that the fissile content of a target spent fuel assembly can be determined using CIPN signal.

  19. Method of assaying uranium with prompt fission and thermal neutron borehole logging adjusted by borehole physical characteristics. [Patient application

    DOEpatents

    Barnard, R.W.; Jensen, D.H.

    1980-11-05

    Uranium formations are assayed by prompt fission neutron logging techniques. The uranium in the formation is proportional to the ratio of epithermal counts to thermal or epithermal dieaway. Various calibration factors enhance the accuracy of the measurement.

  20. Method of assaying uranium with prompt fission and thermal neutron borehole logging adjusted by borehole physical characteristics

    DOEpatents

    Barnard, Ralston W.; Jensen, Dal H.

    1982-01-01

    Uranium formations are assayed by prompt fission neutron logging techniques. The uranium in the formation is proportional to the ratio of epithermal counts to thermal or eqithermal dieaway. Various calibration factors enhance the accuracy of the measurement.

  1. Prompt-gamma neutron activation analysis system design: Effects of D-T versus D-D neutron generator source selection

    Technology Transfer Automated Retrieval System (TEKTRAN)

    Prompt-gamma neutron activation (PGNA) analysis is used for the non-invasive measurement of human body composition. Advancements in portable, compact neutron generator design have made those devices attractive as neutron sources. Two distinct generators are available: D-D with 2.5 MeV and D-T with...

  2. Prompt-gamma neutron activation analysis system design: effects of D-T versus D-D neutron generator source selection

    Technology Transfer Automated Retrieval System (TEKTRAN)

    Prompt-gamma neutron activation analysis (PGNAA) is used for the non-invasive measurement of human body composition. Advancements in portable, compact neutron generator design have made those devices attractive as neutron sources. Two distinct generators are available: D-D with 2.5 MeV, and D-T wi...

  3. Prompt γ rays in 77Ge and 75Ge after thermal neutron capture

    NASA Astrophysics Data System (ADS)

    Meierhofer, G.; Grabmayr, P.; Canella, L.; Kudejova, P.; Jolie, J.; Warr, N.

    2012-02-01

    The reactions 74Ge(n, γ) and 76Ge(n, γ) have been measured with cold neutrons generated by the research reactor FRM II near Munich, Germany. The γ rays have been detected by two Compton-suppressed HPGe systems in single and coincidence mode. The number of identified prompt transitions and levels in 77Ge was increased significantly and the decay scheme could be reconstructed for the first time. The decay scheme was also reconstructed for 68 prompt transitions in 75Ge. Previously reported inconsistencies of the γ-ray intensities in the 77Ge β decay could be resolved. In particular, the region around 2039 keV was investigated carefully, since the background to the neutrinoless double-beta decay of 76Ge must be understood well for the upcoming Gerda and Majorana experiments.

  4. Fast digitization and discrimination of prompt neutron and photon signals using a novel silicon carbide detector

    SciTech Connect

    Brandon W. Blackburn; James T. Johnson; Scott M. Watson; David L. Chichester; James L. Jones; Frank H. Ruddy; John G. Seidel; Robert W. Flammang

    2007-04-01

    Current requirements of some Homeland Security active interrogation projects for the detection of Special Nuclear Material (SNM) necessitate the development of faster inspection and acquisition capabilities. In order to do so, fast detectors which can operate during and shortly after intense interrogation radiation flashes are being developed. Novel silicon carbide (SiC) semiconductor Schottky diodes have been utilized as robust neutron and photon detectors in both pulsed photon and pulsed neutron fields and are being integrated into active inspection environments to allow exploitation of both prompt and delayed emissions. These detectors have demonstrated the capability of detecting both photon and neutron events during intense photon flashes typical of an active inspection environment. Beyond the inherent insensitivity of SiC to gamma radiation, fast digitization and processing has demonstrated that pulse shape discrimination (PSD) in combination with amplitude discrimination can further suppress unwanted gamma signals and extract fast neutron signatures. Usable neutron signals have been extracted from mixed radiation fields where the background has exceeded the signals of interest by >1000:1.

  5. In vivo Prompt Gamma Neutron Activation Analysis Facility for Total Body Nitrogen and Cd

    SciTech Connect

    Munive, Marco; Revilla, Angel; Solis, Jose L.

    2007-10-26

    A Prompt Gamma Neutron Activation Analysis (PGNAA) system has been designed and constructed to measure the total body nitrogen and Cd for in vivo studies. An aqueous solution of KNO{sub 3} was used as phantom for system calibration. The facility has been used to monitor total body nitrogen (TBN) of mice and found that is related to their diet. Some mice swallowed diluted water with Cl{sub 2}Cd, and the presence of Cd was detected in the animals. The minimum Cd concentration that the system can detect was 20 ppm.

  6. Tomographic image of prompt gamma ray from boron neutron capture therapy: A Monte Carlo simulation study

    NASA Astrophysics Data System (ADS)

    Yoon, Do-Kun; Jung, Joo-Young; Jo Hong, Key; Suk Suh, Tae

    2014-02-01

    Purpose of paper is to confirm the feasibility of acquisition of three dimensional single photon emission computed tomography image from boron neutron capture therapy using Monte Carlo simulation. Prompt gamma ray (478 keV) was used to reconstruct image with ordered subsets expectation maximization method. From analysis of receiver operating characteristic curve, area under curve values of three boron regions were 0.738, 0.623, and 0.817. The differences between length of centers of two boron regions and distance of maximum count points were 0.3 cm, 1.6 cm, and 1.4 cm.

  7. Tomographic image of prompt gamma ray from boron neutron capture therapy: A Monte Carlo simulation study

    SciTech Connect

    Yoon, Do-Kun; Jung, Joo-Young; Suk Suh, Tae; Jo Hong, Key

    2014-02-24

    Purpose of paper is to confirm the feasibility of acquisition of three dimensional single photon emission computed tomography image from boron neutron capture therapy using Monte Carlo simulation. Prompt gamma ray (478 keV) was used to reconstruct image with ordered subsets expectation maximization method. From analysis of receiver operating characteristic curve, area under curve values of three boron regions were 0.738, 0.623, and 0.817. The differences between length of centers of two boron regions and distance of maximum count points were 0.3 cm, 1.6 cm, and 1.4 cm.

  8. Prompt Gamma Rays in {sup 77}Ge after Neutron Capture on {sup 76}Ge

    SciTech Connect

    Meierhofer, Georg; Grabmayr, Peter; Jochum, Josef; Canella, Lea; Jolie, Jan; Kudejova, Petra; Warr, Nigel

    2009-01-28

    The observation of neutrinoless double beta decay would be proof of the Majorana nature of the neutrino. Half-lives for these decays are very long (for {sup 76}Ge:>10{sup 25} y), so background reduction and rejection is the major task for double beta experiments. The GERDA (GERmanium Detector Array) experiment at the Gran Sasso Laboratory of the INFN (LNGS) searches for neutrinoless double beta decay of {sup 76}Ge. The isotope {sup 76}Ge is an ideal candidate because it can be used as source and detector at the same time. A large remaining contribution to the background arises from the prompt gamma cascade after neutron capture by {sup 76}Ge followed by {beta}{sup -}-decay of {sup 77}Ge. Since the prompt gamma decay scheme is poorly known, measurements with isotopically enriched Germanium samples were carried out at the PGAA facility at the research reactor FRM II (Munich). With the known prompt gamma spectrum it will be possible to improve the overall veto efficiency of the GERDA experiment.

  9. GPU-based prompt gamma ray imaging from boron neutron capture therapy

    SciTech Connect

    Yoon, Do-Kun; Jung, Joo-Young; Suk Suh, Tae; Jo Hong, Key; Sil Lee, Keum

    2015-01-15

    Purpose: The purpose of this research is to perform the fast reconstruction of a prompt gamma ray image using a graphics processing unit (GPU) computation from boron neutron capture therapy (BNCT) simulations. Methods: To evaluate the accuracy of the reconstructed image, a phantom including four boron uptake regions (BURs) was used in the simulation. After the Monte Carlo simulation of the BNCT, the modified ordered subset expectation maximization reconstruction algorithm using the GPU computation was used to reconstruct the images with fewer projections. The computation times for image reconstruction were compared between the GPU and the central processing unit (CPU). Also, the accuracy of the reconstructed image was evaluated by a receiver operating characteristic (ROC) curve analysis. Results: The image reconstruction time using the GPU was 196 times faster than the conventional reconstruction time using the CPU. For the four BURs, the area under curve values from the ROC curve were 0.6726 (A-region), 0.6890 (B-region), 0.7384 (C-region), and 0.8009 (D-region). Conclusions: The tomographic image using the prompt gamma ray event from the BNCT simulation was acquired using the GPU computation in order to perform a fast reconstruction during treatment. The authors verified the feasibility of the prompt gamma ray image reconstruction using the GPU computation for BNCT simulations.

  10. Event-by-event evaluation of the prompt fission neutron spectrum from 239Pu(n,f)

    NASA Astrophysics Data System (ADS)

    Vogt, R.; Randrup, J.; Brown, D. A.; Descalle, M. A.; Ormand, W. E.

    2012-02-01

    Earlier studies of 239Pu(n,f) have been extended to incident neutron energies up to 20 MeV within the framework of the event-by-event fission model FREYA, into which we have incorporated multichance fission and pre-equilibrium neutron emission. The main parameters controlling prompt fission neutron evaporation have been identified and the prompt fission neutron spectrum has been analyzed by fitting those parameters to the average neutron multiplicity ν¯ from ENDF-B/VII.0, including the energy-energy correlations in the covariance of ν¯(E) obtained by fitting to the experimental ν¯ data used in the ENDF-B/VII.0 evaluation. We present our results, discuss relevant tests of this new evaluation, and describe possible further improvements.

  11. Accurate evolutions of inspiralling neutron-star binaries: Prompt and delayed collapse to a black hole

    NASA Astrophysics Data System (ADS)

    Baiotti, Luca; Giacomazzo, Bruno; Rezzolla, Luciano

    2008-10-01

    Binary neutron-star systems represent primary sources for the gravitational-wave detectors that are presently operating or are close to being operating at the target sensitivities. We present a systematic investigation in full general relativity of the dynamics and gravitational-wave emission from binary neutron stars which inspiral and merge, producing a black hole surrounded by a torus. Our results represent the state of the art from several points of view: (i) We use high-resolution shock-capturing methods for the solution of the hydrodynamics equations and high-order finite-differencing techniques for the solution of the Einstein equations; (ii) We employ adaptive mesh-refinement techniques with “moving boxes” that provide high-resolution around the orbiting stars; (iii) We use as initial data accurate solutions of the Einstein equations for a system of binary neutron stars in irrotational quasicircular orbits; (iv) We exploit the isolated-horizon formalism to measure the properties of the black holes produced in the merger; (v) Finally, we use two approaches, based either on gauge-invariant perturbations or on Weyl scalars, to calculate the gravitational waves emitted by the system. Within our idealized treatment of the matter, these techniques allow us to perform accurate evolutions on time scales never reported before (i.e. ˜30ms) and to provide the first complete description of the inspiral and merger of a neutron-star binary leading to the prompt or delayed formation of a black hole and to its ringdown. We consider either a polytropic equation of state or that of an ideal fluid and show that already with this idealized treatment a very interesting phenomenology can be described. In particular, we show that while higher-mass polytropic binaries lead to the prompt formation of a rapidly rotating black hole surrounded by a dense torus, lower-mass binaries give rise to a differentially rotating star, which undergoes large oscillations and emits large

  12. Imaging of heterogeneous materials by prompt gamma-ray neutron activation analysis

    SciTech Connect

    Staples, P.; Prettyman, T.; Lestone, J.

    1998-12-01

    The authors have used a tomographic gamma scanner (TGS) to produce tomographic prompt gamma-ray neutron activation analysis imaging (PGNAA) of heterogeneous matrices. The TGS was modified by the addition of graphite reflectors that contain isotopic neutron sources for sample interrogation. The authors are in the process of developing the analysis methodology necessary for a quantitative assay of large containers of heterogeneous material. This nondestructive analysis (NDA) technique can be used for material characterization and the determination of neutron assay correction factors. The most difficult question to be answered is the determination of the source-to-sample coupling term. To assist in the determination of the coupling term, the authors have obtained images for a range of sample that are very well characterized, such as, homogenous pseudo one-dimensional samples to three-dimensional heterogeneous samples. They then compare the measurements to MCNP calculations. For an accurate quantitative measurement, it is also necessary to determine the sample gamma-ray self attenuation at higher gamma-ray energies, namely pair production should be incorporated into the analysis codes.

  13. Feasibility study of prompt gamma neutron activation for NDT measurement of moisture in stone and brick

    SciTech Connect

    Livingston, R. A.; Al-Sheikhly, M.; Grissom, C.; Aloiz, E.; Paul, R.

    2014-02-18

    The conservation of stone and brick architecture or sculpture often involves damage caused by moisture. The feasibility of a NDT method based on prompt gamma neutron activation (PGNA) for measuring the element hydrogen as an indication of water is being evaluated. This includes systematic characterization of the lithology and physical properties of seven building stones and one brick type used in the buildings of the Smithsonian Institution in Washington, D.C. To determine the required dynamic range of the NDT method, moisture-related properties were measured by standard methods. Cold neutron PGNA was also used to determine chemically bound water (CBW) content. The CBW does not damage porous masonry, but creates an H background that defines the minimum level of detection of damaging moisture. The CBW was on the order of 0.5% for all the stones. This rules out the measurement of hygric processes in all of the stones and hydric processed for the stones with fine scale pore-size distributions The upper bound of moisture content, set by porosity through water immersion, was on the order of 5%. The dynamic range is about 10–20. The H count rates were roughly 1–3 cps. Taking into account differences in neutron energies and fluxes and sample volume between cold PGNA and a portable PGNA instrument, it appears that it is feasible to apply PGNA in the field.

  14. 239Pu Prompt Fission Neutron Spectra Impact on a Set of Criticality and Experimental Reactor Benchmarks

    NASA Astrophysics Data System (ADS)

    Peneliau, Y.; Litaize, O.; Archier, P.; De Saint Jean, C.

    2014-04-01

    A large set of nuclear data are investigated to improve the calculation predictions of the new neutron transport simulation codes. With the next generation of nuclear power plants (GEN IV projects), one expects to reduce the calculated uncertainties which are mainly coming from nuclear data and are still very important, before taking into account integral information in the adjustment process. In France, future nuclear power plant concepts will probably use MOX fuel, either in Sodium Fast Reactors or in Gas Cooled Fast Reactors. Consequently, the knowledge of 239Pu cross sections and other nuclear data is crucial issue in order to reduce these sources of uncertainty. The Prompt Fission Neutron Spectra (PFNS) for 239Pu are part of these relevant data (an IAEA working group is even dedicated to PFNS) and the work presented here deals with this particular topic. The main international data files (i.e. JEFF-3.1.1, ENDF/B-VII.0, JENDL-4.0, BRC-2009) have been considered and compared with two different spectra, coming from the works of Maslov and Kornilov respectively. The spectra are first compared by calculating their mathematical moments in order to characterize them. Then, a reference calculation using the whole JEFF-3.1.1 evaluation file is performed and compared with another calculation performed with a new evaluation file, in which the data block containing the fission spectra (MF=5, MT=18) is replaced by the investigated spectra (one for each evaluation). A set of benchmarks is used to analyze the effects of PFNS, covering criticality cases and mock-up cases in various neutron flux spectra (thermal, intermediate, and fast flux spectra). Data coming from many ICSBEP experiments are used (PU-SOL-THERM, PU-MET-FAST, PU-MET-INTER and PU-MET-MIXED) and French mock-up experiments are also investigated (EOLE for thermal neutron flux spectrum and MASURCA for fast neutron flux spectrum). This study shows that many experiments and neutron parameters are very sensitive to

  15. Stabilization of prompt gamma-ray neutron activation analysis (PGNAA) spectra from NaI detectors

    NASA Astrophysics Data System (ADS)

    Metwally, W. A.; Gardner, R. P.

    2004-06-01

    NaI detectors are still used frequently in industrial Prompt Gamma-Ray Neutron Activation Analysis applications such as in bulk material analysis. They have the advantages of being efficient for high-energy gamma rays, being relatively rugged, and being able to be used without cooling. When using NaI detectors, and consequently photomultiplier tubes, the quality of the data can drastically deteriorate through gain and zero shifts that result in spectral smearing due to temperature and/or counting rate changes. A new offline approach is presented to stabilize the NaI spectral drift. The approach is not sensitive to the cause of the drift and takes into account the NaI and ADC non-linearities. Peak resolution is improved substantially when this approach is used in the presence of spectral drift.

  16. The optimization of gamma spectra processing in prompt gamma neutron activation analysis (PGNAA)

    NASA Astrophysics Data System (ADS)

    Pinault, Jean-Louis; Solis, Jose

    2009-04-01

    The uncertainty of the elemental analysis is one of the major factors governing the utility of on-line Prompt Gamma Neutron Activation Analysis (PGNAA) in the blending and sorting of bulk materials. In this paper, a general method applicable to Gamma spectra processing is presented and applied to PGNAA in mineral industry. Based on the Fourier transform of spectra and their de-correlation in the Fourier space (the improvement of the conditioning of the correlation matrix), processing of overlapping of characteristic peaks minimizes the propagation of random errors, which optimizes the accuracy and decreases the detection limits of elemental analyses. In comparison with classical methods based on the linear combinations of relevant regions of spectra the improvement may be considerable, especially when several elements are interfering. The method is applied to four case stories covering both borehole logging and on-line analysis on conveyor belt of raw materials.

  17. Fission cross-sections, prompt fission neutron and γ-ray emission in request for nuclear applications

    NASA Astrophysics Data System (ADS)

    Hambsch, F.-J.; Salvador-Castiñeira, P.; Oberstedt, S.; Göök, A.; Billnert, R.

    2016-06-01

    In recent years JRC-IRMM has been investigating fission cross-sections of 240,242Pu in the fast-neutron energy range relevant for innovative reactor systems and requested in the High Priority Request List (HPRL) of the OECD/Nuclear Energy Agency (NEA). In addition to that, prompt neutron multiplicities are being investigated for the major isotopes 235U, 239Pu in the neutron-resonance region using a newly developed scintillation detector array (SCINTIA) and an innovative modification of the Frisch-grid ionisation chamber for fission-fragment detection. These data are highly relevant for improved neutron data evaluation and requested by the OECD/Working Party on Evaluation Cooperation (WPEC). Thirdly, also prompt fission γ-ray emission is investigated using highly efficient lanthanide-halide detectors with superior timing resolution. Again, those data are requested in the HPRL for major actinides to solve open questions on an under-prediction of decay heat in nuclear reactors. The information on prompt fission neutron and γ-ray emission is crucial for benchmarking nuclear models to study the de-excitation process of neutron-rich fission fragments. Information on γ-ray emission probabilities is also useful in decommissioning exercises on damaged nuclear power plants like Fukushima Daiichi to which JRC-IRMM is contributing. The results on the 240,242Pu fission cross section, 235U prompt neutron multiplicity in the resonance region and correlations with fission fragments and prompt γ-ray emission for several isotopes will be presented and put into perspective.

  18. In-vivo assessment of total body protein in rats by promptneutron activation analysis

    NASA Astrophysics Data System (ADS)

    Stamatelatos, Ion E.; Boozer, Carol N.; Ma, Ruimei; Yasumura, Seiichi

    1997-02-01

    A prompt-(gamma) neutron activation analysis facility for in vivo determination of total body protein (TBP) in rats has been designed. TBP is determined in vivo by assessment of total body nitrogen. The facility is based on a 252Cf radionuclide neutron source within a heavy water moderator assembly and two NaI(Tl) scintillation detectors. The in vivo precision of the technique, as estimated by three repeated measurements of 15 rats is 6 percent, for a radiation dose equivalent of 60 mSv. The radiation dose per measurement is sufficiently low to enable serial measurements on the same animal. MCNP-4A Monte Carlo transport code was utilized to calculate thermal neutron flux correction factors to account for differences in size and shape of the rats and calibration phantoms. Good agrement was observed in comparing body nitrogen assessment by prompt-(gamma) neutron activation and chemical carcass analysis.

  19. Fission Mode Influence on Prompt Neutrons and γ-rays Emitted in the Reaction 239Pu(nth,f)

    NASA Astrophysics Data System (ADS)

    Serot, O.; Litaize, O.; Regnier, D.

    Recently, a Monte-Carlo code, which simulates the fission fragment de-excitation process, has been developed at CEA- Cadarache. Our aim is to get a tool capable to predict spectra and multiplicities of prompt particles (neutron and gamma) and to investigate possible correlations between fission observables. One of the main challenges is to define properly the share of the available excitation energy at scission between the two nascent fission fragments. Initially, after the full acceleration of the fission fragments, these excitation energies were treated within a Fermi-gas approximation in aT2 (where a and T stand for the level density parameter and the nuclear temperature) and a mass dependent law of the temperature ratio (RT=TL/TH, with TL and TH the temperature of the light and heavy fragment) has been proposed. With this RT-law, the main fission observables of the 252Cf(sf) could be reproduced. Here, in order to take into account the fission modes by which the fissioning nucleus undergoes to fission, we have adopted a specific RT-law for each fission mode. For actinides, the main fission modes are called Standard I, Standard II and Super Long (following Brosa's terminology). This new procedure has been applied in the case of the thermal neutron induced fission of 239Pu, reaction for which fission modes are rather well known.

  20. Determination of hydrogen in metals, semiconductors, and other materials by cold neutron prompt gamma-ray activation analysis

    SciTech Connect

    Paul, R.L.; Lindstrom, R.M.

    1998-12-31

    Cold neutron prompt gamma-ray activation analysis has proven useful for nondestructive measurement of trace hydrogen. The sample is irradiated in a beam of neutrons; the presence of hydrogen is confirmed by the emission of a 2223 keV gamma-ray. Detection limits for hydrogen are 3 mg/kg in quartz and 8 mg/kg in titanium. The authors have used the technique to measure hydrogen in titanium alloys, germanium, quartz, fullerenes and their derivatives, and other materials.

  1. Improved Modeling of Prompt Fission Neutron Spectra for Nuclear Data Evaluations

    NASA Astrophysics Data System (ADS)

    Neudecker, Denise; Talou, Patrick; Kawano, Toshihiko; Kahler, Albert C.; White, Morgan C.

    2015-10-01

    The prompt fission neutron spectra (PFNS) of major actinides such as 239Pu and 235U are quantities of interest for nuclear physics application areas including reactor physics and national security. Nuclear data evaluations provide recommended data for those application areas based on nuclear theory and experiments. Here, we present improvements made to the effective models predicting the PFNS up to incident neutron energies of 30 MeV and their impact on evaluations. These models describe relevant physics processes better than those used for the current US nuclear data library ENDF/B-VII.1. In addition, the use of higher-fidelity models such as Monte Carlo Hauser-Feshbach calculations will be discussed in the context of future PFNS evaluations. (LA-UR-15-24763) This work was carried out under the auspices of the US Department of Energy, National Nuclear Security Administration and Office of Science, and performed by Los Alamos National Security LLC under Contract DE-AC52-06NA25396.

  2. Thermal-neutron-capture prompt-gamma emission spectra of representative coals. [1. 5 to 11 MeV

    SciTech Connect

    Herzenberg, C L; Olson, I K

    1981-12-01

    Prompt gamma ray emission spectra have been calculated from 1.5 to 11 MeV for a wide range of coal compositions exposed to a thermal neutron flux. These include contributions to the spectra from all of the major and minor elements present in the coals. Characteristics of the spectra are discussed and correlated with the coal compositions.

  3. COHN analysis: Body composition measurements based on the associated particle imaging and prompt-gamma neutron activation analysis techniques

    Technology Transfer Automated Retrieval System (TEKTRAN)

    The measurement of the body's carbon (C), oxygen (O), hydrogen (H), and nitrogen (N) content can be used to calculate the relative amounts of fat, protein, and water. A system based on prompt-gamma neutron activation analysis (PGNAA), coupled with the associated particle imaging (API) technique, is...

  4. Determination and validation of prompt k0-factors with a monochromatic neutron beam at the Dhruva reactor

    NASA Astrophysics Data System (ADS)

    Nair, A. G. C.; Acharya, R.; Sudarshan, K.; Tripathi, R.; Reddy, A. V. R.; Goswami, A.

    2006-08-01

    Prompt Gamma-ray Neutron Activation Analysis (PGNAA) was carried out using a reflected neutron beam of 0.018 eV energy at the Dhruva research reactor, Bhabha Atomic Research Centre, Mumbai, India. The neutron beam characteristics, such as dimension, homogeneity and thermal equivalent flux were evaluated. The prompt k0-factors of about 15 elements were determined versus the 1951.1 keV gamma-ray of the 35Cl(n,γ) reaction. These prompt k0-factors are compared with the recommended k0-values for thermal neutrons and were found to be in good agreement, except for Gd, Cd and Hg. The internal mono-standard method was applied to analyze a meteorite and a stainless steel alloy (SS 316 M) using the recommended k0-values from the literature. As to the alloy, the measured concentrations were in good agreement with the nominal composition. For the meteorite sample, the concentrations of the major elements were in good agreement with the values determined using conventional neutron activation analysis.

  5. Preliminary Results of a Full Hauser-feshbach Simulation of the Prompt Neutron and Gamma Emission from Fission Fragments

    NASA Astrophysics Data System (ADS)

    Regniera, D.; Litaizea, O.; Serota, O.

    The prompt neutron and gamma emission from fission fragments are investigated through the Monte Carlo code FIFRELIN which is developed at the CEA Cadarache research center. In a previous release of the code, the de-excitation of the fragments was treated in a two steps process. First the emission of all the prompt neutrons was simulated using a Weisskopf spectrum for the distribution of their kinetic energy. In a second step, the excitation energy still available was dissipated by the fragments as an electromagnetic decay cascade. This paper presents a new procedure for fragment de-excitation using an Hauser-Feshbach treatment of prompt particles emission. The neutron/gamma competition is then accounted for during the whole cascade. Moreover, the neutron emission is now ruled by the transmission coefficients directly coming from an optical model calculation performed with TALYS-1.4. The implementation of these models in the code FIFRELIN is quickly highlighted. The results in terms of neutrons and gamma multiplicities and spectra for one simulation of a 252Cf spontaneous fission are emphasized. The neutron multiplicity experimental data are used to constraint the parameters of our simulation. The prompt gamma spectrum calculated is then consistent with experimental data and the structures observed experimentally in the low energy range are well reproduced. However, the same simulation performed with several different nuclear models and parameters reveals high variation of these fission observables. For example, the average total gamma energy (Eγ,tot) is shown to vary up to 20% with changes in the level density or radiative strength function model.

  6. Angular Correlations Between Fragment Spin and Prompt Neutron Evaporation in Spontaneous Fission of 252Cf: CORA-Demon Experiment

    SciTech Connect

    Prokhorova, E.; Goennenwein, F.; Kopatch, Yu.; Mutterer, M.; Hanappe, F.; Kinnard, V.; Stuttge, L.; Dorvaux, O.; Wollersheim, H.-J.

    2007-05-22

    A novel method to search for the anisotropic emission of prompt neutrons in the center-of-mass system of fission fragments is presented. The anisotropy is conjectured to be due to the large spins of fission fragments are known to carry. Triple neutron- neutron-fragment correlations in spontaneous fission of 252Cf were investigated in an exploratory experiment dubbed CORA-DEMON experiment. Fission fragments were intercepted in a double ionization chamber while neutrons were spotted in 2 two-dimensional cylindrical walls of Demon detectors with the target on the vertical cylinder axis. A new method of analysis of triple angular correlations between 2 neutrons and a fission fragment was applied. Preliminary results are reported.

  7. Angular Correlations Between Fragment Spin and Prompt Neutron Evaporation in Spontaneous Fission of 252Cf: CORA-Demon Experiment

    NASA Astrophysics Data System (ADS)

    Prokhorova, E.; Gönnenwein, F.; Kopatch, Yu.; Mutterer, M.; Hanappe, F.; Kinnard, V.; Stuttgé, L.; Dorvaux, O.; Wollersheim, H.-J.

    2007-05-01

    A novel method to search for the anisotropic emission of prompt neutrons in the center-of-mass system of fission fragments is presented. The anisotropy is conjectured to be due to the large spins of fission fragments are known to carry. Triple neutron- neutron-fragment correlations in spontaneous fission of 252Cf were investigated in an exploratory experiment dubbed CORA-DEMON experiment. Fission fragments were intercepted in a double ionization chamber while neutrons were spotted in 2 two-dimensional cylindrical walls of Demon detectors with the target on the vertical cylinder axis. A new method of analysis of triple angular correlations between 2 neutrons and a fission fragment was applied. Preliminary results are reported.

  8. Prompt gamma neutron activation analysis of toxic elements in radioactive waste packages.

    PubMed

    Ma, J-L; Carasco, C; Perot, B; Mauerhofer, E; Kettler, J; Havenith, A

    2012-07-01

    The French Alternative Energies and Atomic Energy Commission (CEA) and National Radioactive Waste Management Agency (ANDRA) are conducting an R&D program to improve the characterization of long-lived and medium activity (LL-MA) radioactive waste packages. In particular, the amount of toxic elements present in radioactive waste packages must be assessed before they can be accepted in repository facilities in order to avoid pollution of underground water reserves. To this aim, the Nuclear Measurement Laboratory of CEA-Cadarache has started to study the performances of Prompt Gamma Neutron Activation Analysis (PGNAA) for elements showing large capture cross sections such as mercury, cadmium, boron, and chromium. This paper reports a comparison between Monte Carlo calculations performed with the MCNPX computer code using the ENDF/B-VII.0 library and experimental gamma rays measured in the REGAIN PGNAA cell with small samples of nickel, lead, cadmium, arsenic, antimony, chromium, magnesium, zinc, boron, and lithium to verify the validity of a numerical model and gamma-ray production data. The measurement of a ∼20kg test sample of concrete containing toxic elements has also been performed, in collaboration with Forschungszentrum Jülich, to validate the model in view of future performance studies for dense and large LL-MA waste packages. PMID:22406218

  9. Uncertainty Quantification of Prompt Fission Neutron Spectra Using the Unified Monte Carlo Method

    NASA Astrophysics Data System (ADS)

    Rising, M. E.; Talou, P.; Prinja, A. K.

    2014-04-01

    In the ENDF/B-VII.1 nuclear data library, the existing covariance evaluations of the prompt fission neutron spectra (PFNS) were computed by combining the available experimental differential data with theoretical model calculations, relying on the use of a first-order linear Bayesan approach, the Kalman filter. This approach assumes that the theoretical model response to changes in input model parameters be linear about the a priori central values. While the Unified Monte Carlo (UMC) method remains a Bayesian approach, like the Kalman filter, this method does not make any assumption about the linearity of the model response or shape of the a posteriori distribution of the parameters. By sampling from a distribution centered about the a priori model parameters, the UMC method computes the moments of the a posteriori parameter distribution. As the number of samples increases, the statistical noise in the computed a posteriori moments decrease and an appropriately converged solution corresponding to the true mean of the a posteriori PDF results. The UMC method has been successfully implemented using both a uniform and Gaussian sampling distribution and has been used for the evaluation of the PFNS and its associated uncertainties. While many of the UMC results are similar to the first-order Kalman filter results, significant differences are shown when experimental data are excluded from the evaluation process. When experimental data are included a few small nonlinearities are present in the high outgoing energy tail of the PFNS.

  10. Feasibility study of prompt gamma neutron activation analysis (PGNAA) of explosives simulants and bulk material using DD/DT neutron generator

    NASA Astrophysics Data System (ADS)

    Bishnoi, S.; Sarkar, P. S.; Patel, T.; Adhikari, P. S.; Sinha, Amar

    2013-04-01

    Elemental characterization of low Z elements (C,H,Cl,Fe) inside bulk materials were performed using PGNAA technique. Samples having elemental composition similar to explosives were used for such experimentations using moderated DD neutrons as well as DT(14MeV) neutrons. We could observe characteristic prompt capture gamma rays of hydrogen (2.224MeV), nitrogen (10.83 MeV), chlorine (6.11 MeV) and Fe (6.02MeV and 7.63MeV) also (n,n'γ) prompt gamma signal (4.43MeV) of carbon. BGO detector has been used for gamma spectrum acquisition. These experimentations has been carried out for initial feasibility studies of detecting prompt gamma lines as a part of PGNAA technique based explosive detection system development. A detail description of experimental set up and procedure has been discussed in paper.

  11. A benchmarked MCNP model of the in vivo detection of gadolinium by prompt gamma neutron activation analysis

    NASA Astrophysics Data System (ADS)

    Gräfe, J. L.; McNeill, F. E.; Byun, S. H.; Chettle, D. R.; Noseworthy, M. D.

    2010-08-01

    Gadolinium (Gd)-based contrast agents are a valuable diagnostic aid for magnetic resonance imaging (MRI). The amount of free Gd deposited in tissues following contrast enhanced MRI is of toxicological concern. The McMaster University in vivo prompt gamma neutron activation analysis facility has been adapted for the detection of Gd in the kidney, liver, and the leg muscle. A simple model of the HPGe detector used for detection of the prompt γ-rays following Gd neutron capture has been created using Monte Carlo simulation. A separate simulation describing the neutron collimation and shielding apparatus has been modified to determine the neutron capture rate in the Gd phantoms. The MCNP simulation results have been confirmed by experimental measurement. The deviations between MCNP and the experiment were between 1% and 18%, with an average deviation of 3.8 ± 6.7%. The validated MCNP model is to be used to improve the Gd in vivo measurement sensitivity by determining the best neutron moderator/reflector arrangement.

  12. Development of a database for prompt gamma-ray neutron activation analysis: Summary report of the third research coordination meeting

    SciTech Connect

    Lindstrom, Richard M.; Firestone, Richard B.; Pavi, ???

    2003-04-01

    The main discussions and conclusions from the Third Co-ordination Meeting on the Development of a Database for Prompt Gamma-ray Neutron Activation Analysis are summarized in this report. All results were reviewed in detail, and the final version of the TECDOC and the corresponding software were agreed upon and approved for preparation. Actions were formulated with the aim of completing the final version of the TECDOC and associated software by May 2003.

  13. Neutron kinetics in moderators and SNM detection through epithermal-neutron-induced fissions

    NASA Astrophysics Data System (ADS)

    Gozani, Tsahi; King, Michael J.

    2016-01-01

    Extension of the well-established Differential Die Away Analysis (DDAA) into a faster time domain, where more penetrating epithermal neutrons induce fissions, is proposed and demonstrated via simulations and experiments. In the proposed method the fissions stimulated by thermal, epithermal and even higher-energy neutrons are measured after injection of a narrow pulse of high-energy 14 MeV (d,T) or 2.5 MeV (d,D) source neutrons, appropriately moderated. The ability to measure these fissions stems from the inherent correlation of neutron energy and time ("E-T" correlation) during the process of slowing down of high-energy source neutrons in common moderating materials such as hydrogenous compounds (e.g., polyethylene), heavy water, beryllium and graphite. The kinetic behavior following injection of a delta-function-shaped pulse (in time) of 14 MeV neutrons into such moderators is studied employing MCNPX simulations and, when applicable, some simple "one-group" models. These calculations served as a guide for the design of a source moderator which was used in experiments. Qualitative relationships between slowing-down time after the pulse and the prevailing neutron energy are discussed. A laboratory system consisting of a 14 MeV neutron generator, a polyethylene-reflected Be moderator, a liquid scintillator with pulse-shape discrimination (PSD) and a two-parameter E-T data acquisition system was set up to measure prompt neutron and delayed gamma-ray fission signatures in a 19.5% enriched LEU sample. The measured time behavior of thermal and epithermal neutron fission signals agreed well with the detailed simulations. The laboratory system can readily be redesigned and deployed as a mobile inspection system for SNM in, e.g., cars and vans. A strong pulsed neutron generator with narrow pulse (<75 ns) at a reasonably high pulse frequency could make the high-energy neutron induced fission modality a realizable SNM detection technique.

  14. Probing energy dissipation, γ-ray and neutron multiplicity in the thermal neutron-induced fission of 239Pu

    NASA Astrophysics Data System (ADS)

    Pahlavani, M. R.; Mirfathi, S. M.

    2016-04-01

    The incorporation of the four-dimensional Langevin equations led to an integrative description of fission cross-section, fragment mass distribution and the multiplicity and energy distribution of prompt neutrons and γ-rays in the thermal neutron-induced fission of 239Pu. The dynamical approach presented in this paper thoroughly reproduces several experimental observables of the fission process at low excitation energy.

  15. Verification of threshold activation detection (TAD) technique in prompt fission neutron detection using scintillators containing 19F

    NASA Astrophysics Data System (ADS)

    Sibczynski, P.; Kownacki, J.; Moszyński, M.; Iwanowska-Hanke, J.; Syntfeld-Każuch, A.; Gójska, A.; Gierlik, M.; Kaźmierczak, Ł.; Jakubowska, E.; Kędzierski, G.; Kujawiński, Ł.; Wojnarowicz, J.; Carrel, F.; Ledieu, M.; Lainé, F.

    2015-09-01

    In the present study ⌀ 5''× 3'' and ⌀ 2''× 2'' EJ-313 liquid fluorocarbon as well as ⌀ 2'' × 3'' BaF2 scintillators were exposed to neutrons from a 252Cf neutron source and a Sodern Genie 16GT deuterium-tritium (D+T) neutron generator. The scintillators responses to β- particles with maximum endpoint energy of 10.4 MeV from the n+19F reactions were studied. Response of a ⌀ 5'' × 3'' BC-408 plastic scintillator was also studied as a reference. The β- particles are the products of interaction of fast neutrons with 19F which is a component of the EJ-313 and BaF2 scintillators. The method of fast neutron detection via fluorine activation is already known as Threshold Activation Detection (TAD) and was proposed for photofission prompt neutron detection from fissionable and Special Nuclear Materials (SNM) in the field of Homeland Security and Border Monitoring. Measurements of the number of counts between 6.0 and 10.5 MeV with a 252Cf source showed that the relative neutron detection efficiency ratio, defined as epsilonBaF2 / epsilonEJ-313-5'', is 32.0% ± 2.3% and 44.6% ± 3.4% for front-on and side-on orientation of the BaF2, respectively. Moreover, the ⌀ 5'' EJ-313 and side-on oriented BaF2 were also exposed to neutrons from the D+T neutron generator, and the relative efficiency epsilonBaF2 / epsilonEJ-313-5'' was estimated to be 39.3%. Measurements of prompt photofission neutrons with the BaF2 detector by means of data acquisition after irradiation (out-of-beam) of nuclear material and between the beam pulses (beam-off) techniques were also conducted on the 9 MeV LINAC of the SAPHIR facility.

  16. Systematics of the mean energy and the mean multiplicity of prompt neutrons originating from {sup 232}Th fission

    SciTech Connect

    Svirin, M. I.

    2012-12-15

    The cross section for the neutron-induced fission of {sup 232}Th target nuclei, {sigma}{sub f} (E{sub n}), was described within statistical theory. The spectra of the mean multiplicity, v-bar (E{sub n}), and the mean energy, E-bar(E{sub n}), of secondary neutrons accompanying {sup 232}Th fission induced by neutrons of energy extending up to E{sub n} = 20 MeV were analyzed on the basis of the chance structure of the cross section.

  17. The Prompt Fission Neutron Spectrum: From Experiment to the Evaluated Data and its Impact on Critical Assemblies

    SciTech Connect

    Rising, Michael Evan

    2015-06-10

    After a brief introduction concerning nuclear data, prompt fission neutron spectrum (PFNS) evaluations and the limited PFNS covariance data in the ENDF/B-VII library, and the important fact that cross section uncertainties ~ PFNS uncertainties, the author presents background information on the PFNS (experimental data, theoretical models, data evaluation, uncertainty quantification) and discusses the impact on certain well-known critical assemblies with regard to integral quantities, sensitivity analysis, and uncertainty propagation. He sketches recent and ongoing research and concludes with some final thoughts.

  18. Prompt Neutron Emission from Fragments in Spontaneous Fission of 244, 248Cm and 252Cf

    NASA Astrophysics Data System (ADS)

    Vorobyev, A. S.; Dushin, V. N.; Hambsch, F.-J.; Jakovlev, V. A.; Kalinin, V. A.; Laptev, A. B.; Petrov, B. F.; Shcherbakov, O. A.

    2005-11-01

    Neutrons emitted in fission were measured separately for each complementary fragment in correlation with fission fragment energies. Two high efficient Gd-loaded liquid scintillator tanks were used for neutron registration. Fission fragment energies were measured using a twin Frisch gridded ionization chamber with a pin-hole collimator. The neutron multiplicity distributions were obtained for each value of the fission fragment mass and energy and corrected for neutron registration efficiency, background and pile-up. The dependencies of these distributions on fragment mass and energy for different energy and mass bins, as well as the mass and energy distribution of the fission fragments are presented and discussed.

  19. Prompt neutron emission from the spontaneous fission of sup 260 Md

    SciTech Connect

    Wild, J.F.; van Aarle, J.; Westmeier, W.; Lougheed, R.W.; Hulet, E.K.; Moody, K.J.; Dougan, R.J.; Koop, E.; Glaser, R.E.; Brandt, R.; Patzelt, P. Philipps University, D-3550, Marburg an der Lahn, )

    1990-02-01

    We have made the first measurement of the number of neutrons emitted from the spontaneous fission of a nuclide in which very high fragment energies dominate the fission process. In bombardments of {sup 254}Es, we produced a large sample of 28-d {sup 260}Md, which was neutron counted in a 1-m-diameter spherical tank containing a Gd-doped scintillator solution. The average number of neutrons emitted per fission is only 2.58{plus minus}0.11, substantially less than for other actinides. A linear dependence of neutron multiplicity on fragment-excitation energy is observed to the highest values of total kinetic energy.

  20. Neutron radiography and neutron-induced autoradiography for the classroom

    SciTech Connect

    Aderhold, H.C. )

    1992-01-01

    The Cornell 500-kW MARK II TRIGA reactor at the Ward Laboratory of Nuclear Engineering has been used to illustrate the application of neutron radiography (NR) and neutron-induced autoradiography (NIAR) for solving problems in engineering as well as problems in art history. The applications are described in the paper.

  1. Event-by-event evaluation of the prompt fission neutron spectrum from 239Pu(n,f)

    SciTech Connect

    Vogt, R; Randrup, J; Brown, D A; Descalle, M A; Ormand, W E

    2011-11-28

    We have developed an improved evaluation method for the spectrum of neutrons emitted in fission of {sup 239}Pu induced by incident neutrons with energies up to 20 MeV. The covariance data, including incident energy correlations introduced by the evaluation method, were used to fix the input parameters in our event-by-event model of fission, FREYA, by applying formal statistical methods. Formal estimates of uncertainties in the evaluation were developed by randomly sampling model inputs and calculating likelihood functions based on agreement with the evaluated . Our approach is able to employ a greater variety of fission measurements than the relatively coarse spectral data alone. It also allows the study of numerous fission observables for more accurate model validation. The combination of an event-by-event Monte Carlo fission model with a statistical-likelihood analysis is thus a powerful tool for evaluation of fission-neutron data. Our empirical model FREYA follows the complete fission event from birth of the excited fragments through their decay via neutron emission until the fragment excitation energy is below the neutron separation energy when neutron emission can no longer occur. The most recent version of FREYA incorporates pre-equilibrium neutron emission, the emission of the first neutron before equilibrium is reached in the compound nucleus, and multi-chance fission, neutron evaporation prior to fission when the incident neutron energy is above the neutron separation energy. Energy, momentum, charge and mass number are conserved throughout the fission process. The best available values of fragment masses and total kinetic energies are used as inputs to FREYA. We fit three parameters that are not well under control from previous measurements: the shift in the total fragment kinetic energy; the energy scale of the asymptotic level density parameter, controlling the fragment 'temperature' for neutron evaporation; and the relative excitation of the

  2. Study on Prompt Fission Neutron Spectra and Associated Covariances for 235U(nth,f) and 239Pu(nth,f)

    NASA Astrophysics Data System (ADS)

    Berge, L.; Litaize, O.; Serot, O.; Jean, C. De Saint; Archier, P.; Peneliau, Y.

    Prompt Fission Neutron Spectra (PFNS) are very important nuclear data for reactor neutronic calculation tools. Most of the international evaluated nuclear data libraries lie on the Madland-Nix model, which is a based on evaporation theory of fission fragments. But very scarce data can be found regarding the PFNS covariance matrix associated to these evaluations. As an illustration of the impact of the PFNS on neutronic calculations, we will show a Monte-Carlo calculation of the neutron flux received by a PWR vessel, using different PFNS evaluations. The neutrons that have the highest probability to contribute to the vessel flux are those that are emitted at the highest energies; however most of the fission neutrons are emitted around 2 MeV. These results show the necessity to have very precise PFNS evaluations, and a proper estimation of associated covariances. The estimation of the PFNS covariance matrix associated to a model, after adjustment of model parameters, will be shown. This is performed by the CONRAD code, developed at CEA Cadarache. The final goal of the study is to adjust the parameters involved in fission fragments de-excitation in the FIFRELIN Monte-Carlo code, also developed at CEA Cadarache, which computes the PFNS among other fission quantities, and to provide the associated PFNS covariance matrix. However for the moment we focused the study on three historically widely used PFNS models: Maxwellian, Watt and Madland-Nix models. The covariance matrix on the adjusted spectrum comes mainly from the systematic uncertainty on some experimental parameters - namely the normalization, background, detection efficiency, etc. In order to propagate this type of uncertainties properly, the marginalization technique is used. A close knowledge of the conditions in which a particular experimental PFNS has been measured is required, in order to have a correct estimation of the PFNS uncertainties after adjustment. In this work, we propagated the uncertainty on

  3. In vivo prompt gamma neutron activation analysis for the screening of boron-10 distribution in a rabbit knee: a simulation study

    NASA Astrophysics Data System (ADS)

    Zhu, X.; Clackdoyle, R.; Shortkroff, S.; Yanch, J.

    2008-05-01

    Boron neutron capture synovectomy (BNCS) is under development as a potential treatment modality for rheumatoid arthritis (RA). RA is characterized by the inflammation of the synovium (the membrane lining articular joints), which leads to pain and a restricted range of motion. BNCS is a two-part procedure involving the injection of a boronated compound directly into the diseased joint followed by irradiation with a low-energy neutron beam. The neutron capture reactions taking place in the synovium deliver a local, high-linear energy transfer (LET) dose aimed at destroying the inflamed synovial membrane. For successful treatment via BNCS, a boron-labeled compound exhibiting both high synovial uptake and long retention time is necessary. Currently, the in vivo uptake behavior of potentially useful boronated compounds is evaluated in the knee joints of rabbits in which arthritis has been induced. This strategy involves the sacrifice and dissection of a large number of animals. An in vivo 10B screening approach is therefore under investigation with the goal of significantly reducing the number of animals needed for compound evaluation via dissection studies. The 'in vivo prompt gamma neutron activation analysis' (IVPGNAA) approach uses a narrow neutron beam to irradiate the knee from several angular positions following the intra-articular injection of a boronated compound whose uptake characteristics are unknown. A high-purity germanium detector collects the 478 keV gamma photons produced by the 10B capture reactions. The 10B distribution in the knee is then reconstructed by solving a system of simultaneous equations using a weighted least squares algorithm. To study the practical feasibility of IVPGNAA, simulation data were generated with the Monte Carlo N-particle transport code. The boron-containing region of a rabbit knee was partitioned into 8 compartments, and the 10B prompt gamma signals were tallied from 16 angular positions. Results demonstrate that for this

  4. In vivo prompt gamma neutron activation analysis for the screening of boron-10 distribution in a rabbit knee: a simulation study.

    PubMed

    Zhu, X; Clackdoyle, R; Shortkroff, S; Yanch, J

    2008-05-21

    Boron neutron capture synovectomy (BNCS) is under development as a potential treatment modality for rheumatoid arthritis (RA). RA is characterized by the inflammation of the synovium (the membrane lining articular joints), which leads to pain and a restricted range of motion. BNCS is a two-part procedure involving the injection of a boronated compound directly into the diseased joint followed by irradiation with a low-energy neutron beam. The neutron capture reactions taking place in the synovium deliver a local, high-linear energy transfer (LET) dose aimed at destroying the inflamed synovial membrane. For successful treatment via BNCS, a boron-labeled compound exhibiting both high synovial uptake and long retention time is necessary. Currently, the in vivo uptake behavior of potentially useful boronated compounds is evaluated in the knee joints of rabbits in which arthritis has been induced. This strategy involves the sacrifice and dissection of a large number of animals. An in vivo (10)B screening approach is therefore under investigation with the goal of significantly reducing the number of animals needed for compound evaluation via dissection studies. The 'in vivo prompt gamma neutron activation analysis' (IVPGNAA) approach uses a narrow neutron beam to irradiate the knee from several angular positions following the intra-articular injection of a boronated compound whose uptake characteristics are unknown. A high-purity germanium detector collects the 478 keV gamma photons produced by the (10)B capture reactions. The (10)B distribution in the knee is then reconstructed by solving a system of simultaneous equations using a weighted least squares algorithm. To study the practical feasibility of IVPGNAA, simulation data were generated with the Monte Carlo N-particle transport code. The boron-containing region of a rabbit knee was partitioned into 8 compartments, and the (10)B prompt gamma signals were tallied from 16 angular positions. Results demonstrate that for

  5. Performance characteristics of a prompt gamma-ray activation analysis (PGAA) system equipped with a new compact D-D neutron generator

    NASA Astrophysics Data System (ADS)

    Park, Yong Joon; Song, Byung Chul; Im, Hee-Jung; Kim, Jong-Yun

    2009-07-01

    A new prompt gamma-ray activation analysis (PGAA) system equipped with a compact deuterium-deuterium (D-D) neutron generator has been developed for fast detection of explosives and chemical warfare agents. The PGAA system was built based on a fully high-voltage-shielded, axial D-D neutron generator with a radio frequency (RF)-driven ion source. The ionic current of the compact neutron generator was determined as a function of the acceleration voltage at various RF powers. Monoenergetic neutrons (2.45 MeV) with a neutron yield of >1×107 n/s were obtained at a deuterium pressure of 8.0 mTorr, an acceleration voltage of 80 kV, and an RF power of 1.1 kW. The performance of the PGAA system was examined by studying the dependence of a prompt gamma-ray count rate on crucial operating parameters.

  6. Monitoring the distribution of prompt gamma rays in boron neutron capture therapy using a multiple-scattering Compton camera: A Monte Carlo simulation study

    NASA Astrophysics Data System (ADS)

    Lee, Taewoong; Lee, Hyounggun; Lee, Wonho

    2015-10-01

    This study evaluated the use of Compton imaging technology to monitor prompt gamma rays emitted by 10B in boron neutron capture therapy (BNCT) applied to a computerized human phantom. The Monte Carlo method, including particle-tracking techniques, was used for simulation. The distribution of prompt gamma rays emitted by the phantom during irradiation with neutron beams is closely associated with the distribution of the boron in the phantom. Maximum likelihood expectation maximization (MLEM) method was applied to the information obtained from the detected prompt gamma rays to reconstruct the distribution of the tumor including the boron uptake regions (BURs). The reconstructed Compton images of the prompt gamma rays were combined with the cross-sectional images of the human phantom. Quantitative analysis of the intensity curves showed that all combined images matched the predetermined conditions of the simulation. The tumors including the BURs were distinguishable if they were more than 2 cm apart.

  7. Neutron induced bystander effect among zebrafish embryos

    NASA Astrophysics Data System (ADS)

    Ng, C. Y. P.; Kong, E. Y.; Kobayashi, A.; Suya, N.; Uchihori, Y.; Cheng, S. H.; Konishi, T.; Yu, K. N.

    2015-12-01

    The present paper reported the first-ever observation of neutron induced bystander effect (NIBE) using zebrafish (Danio rerio) embryos as the in vivo model. The neutron exposure in the present work was provided by the Neutron exposure Accelerator System for Biological Effect Experiments (NASBEE) facility at the National Institute of Radiological Sciences (NIRS), Chiba, Japan. Two different strategies were employed to induce NIBE, namely, through directly partnering and through medium transfer. Both results agreed with a neutron-dose window (20-50 mGy) which could induce NIBE. The lower dose limit corresponded to the threshold amount of neutron-induced damages to trigger significant bystander signals, while the upper limit corresponded to the onset of gamma-ray hormesis which could mitigate the neutron-induced damages and thereby suppress the bystander signals. Failures to observe NIBE in previous studies were due to using neutron doses outside the dose-window. Strategies to enhance the chance of observing NIBE included (1) use of a mono-energetic high-energy (e.g., between 100 keV and 2 MeV) neutron source, and (2) use of a neutron source with a small gamma-ray contamination. It appeared that the NASBEE facility used in the present study fulfilled both conditions, and was thus ideal for triggering NIBE.

  8. Prompt gamma activation analysis (PGAA) and short-lived neutron activation analysis (NAA) applied to the characterization of legacy materials

    SciTech Connect

    Firestone, Richard B; English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Leung, Ka-Ngo; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.

    2008-02-13

    Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents.1-3. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity.

  9. Thoughts on Sensitivity Analysis and Uncertainty Propagation Methods with Respect to the Prompt Fission Neutron Spectrum Impact on Critical Assemblies

    SciTech Connect

    Rising, M.E.

    2015-01-15

    The prompt fission neutron spectrum (PFNS) uncertainties in the n+{sup 239}Pu fission reaction are used to study the impact on several fast critical assemblies modeled in the MCNP6.1 code. The newly developed sensitivity capability in MCNP6.1 is used to compute the k{sub eff} sensitivity coefficients with respect to the PFNS. In comparison, the covariance matrix given in the ENDF/B-VII.1 library is decomposed and randomly sampled realizations of the PFNS are propagated through the criticality calculation, preserving the PFNS covariance matrix. The information gathered from both approaches, including the overall k{sub eff} uncertainty, is statistically analyzed. Overall, the forward and backward approaches agree as expected. The results from a new method appear to be limited by the process used to evaluate the PFNS and is not necessarily a flaw of the method itself. Final thoughts and directions for future work are suggested.

  10. Optimization of combined delayed neutron and differential die-away prompt neutron signal detection for characterization of spent nuclear fuel assemblies

    SciTech Connect

    Blanc, Pauline; Tobin, Stephen J; Croft, Stephen; Menlove, Howard O; Swinhoe, M; Lee, T

    2010-12-02

    The Next Generation Safeguards Initiative (NGSI) of the U.S. Department of Energy (DOE) has funded multiple laboratories and universities to develop a means to accurately quantify the Plutonium (Pu) mass in spent nuclear fuel assemblies and ways to also detect potential diversion of fuel pins. Delayed Neutron (DN) counting provides a signature somewhat more sensitive to {sup 235}U than Pu while Differential Die-Away (DDA) is complementary in that it has greater sensitivity to Pu. The two methods can, with care, be combined into a single instrument which also provides passive neutron information. Individually the techniques cannot robustly quantify the Pu content but coupled together the information content in the signatures enables Pu quantification separate to the total fissile content. The challenge of merging DN and DDA, prompt neutron (PN) signal, capabilities in the same design is the focus of this paper. Other possibilities also suggest themselves, such as a direct measurement of the reactivity (multiplication) by either the boost in signal obtained during the active interrogation itself or by the extension of the die-away profile. In an early study, conceptual designs have been modeled using a neutron detector comprising fission chambers or 3He proportional counters and a {approx}14 MeV neutron Deuterium-Tritium (DT) generator as the interrogation source. Modeling was performed using the radiation transport code Monte Carlo N-Particles eXtended (MCNPX). Building on this foundation, the present paper quantifies the capability of a new design using an array of {sup 3}He detectors together with fission chambers to optimize both DN and PN detections and active characterization, respectively. This new design was created in order to minimize fission in {sup 238}U (a nuisance DN emitter), to use a realistic neutron generator, to reduce the cost and to achieve near spatial interrogation and detection of the DN and PN, important for detection of diversion, all within

  11. Enrico Fermi's Discovery of Neutron-Induced Artificial Radioactivity: Neutrons and Neutron Sources

    NASA Astrophysics Data System (ADS)

    Guerra, Francesco; Leone, Matteo; Robotti, Nadia

    2006-09-01

    We reconstruct and analyze the path leading from James Chadwick’s discovery of the neutron in February 1932 through Frédéric Joliot and Irène Curie’s discovery of artificial radioactivity in January 1934 to Enrico Fermi’s discovery of neutron-induced artificial radioactivity in March 1934. We show, in particular, that Fermi’s innovative construction and use of radon-beryllium neutron sources permitted him to make his discovery.

  12. Neutron Damage in Mechanically-Cooled High-Purity Germanium Detectors for Field-Portable Prompt Gamma Neutron Activation Analysis (PGNAA) Systems

    SciTech Connect

    E.H. Seabury; C.J. Wharton; A.J. Caffrey; J.B. McCabe; C. DeW. Van Siclen

    2013-10-01

    Prompt Gamma Neutron Activation (PGNAA) systems require the use of a gamma-ray spectrometer to record the gamma-ray spectrum of an object under test and allow the determination of the object’s composition. Field-portable systems, such as Idaho National Laboratory’s PINS system, have used standard liquid-nitrogen-cooled high-purity germanium (HPGe) detectors to perform this function. These detectors have performed very well in the past, but the requirement of liquid-nitrogen cooling limits their use to areas where liquid nitrogen is readily available or produced on-site. Also, having a relatively large volume of liquid nitrogen close to the detector can impact some assessments, possibly leading to a false detection of explosives or other nitrogen-containing chemical. Use of a mechanically-cooled HPGe detector is therefore very attractive for PGNAA applications where nitrogen detection is critical or where liquid-nitrogen logistics are problematic. Mechanically-cooled HPGe detectors constructed from p-type germanium, such as Ortec’s trans-SPEC, have been commercially available for several years. In order to assess whether these detectors would be suitable for use in a fielded PGNAA system, Idaho National Laboratory (INL) has been performing a number of tests of the resistance of mechanically-cooled HPGe detectors to neutron damage. These detectors have been standard commercially-available p-type HPGe detectors as well as prototype n-type HPGe detectors. These tests compare the performance of these different detector types as a function of crystal temperature and incident neutron fluence on the crystal.

  13. Prompt radiation-induced conductivity in polyurethane foam and glass microballoons

    SciTech Connect

    Hartman, E. Frederick; Zarick, Thomas Andrew; Sheridan, Timothy J.; Preston, Eric F.

    2014-06-01

    We performed measurements and analyses of the prompt radiation-induced conductivity (RIC) in thin samples of polyurethane foam and glass microballoon foam at the Little Mountain Medusa LINAC facility in Ogden, UT. The RIC coefficient was non-linear with dose rate for polyurethane foam; however, typical values at 1E11 rad(si)/s dose rate was measured as 0.8E-11 mho/m/rad/s for 5 lb./cu ft. foam and 0.3E-11 mho/m/rad/s for 10 lb./cu ft. density polyurethane foam. For encapsulated glass microballoons (GMB) the RIC coefficient was approximately 1E-15 mho/m/rad/s and was not a strong function of dose rate.

  14. Toward prompt gamma spectrometry for monitoring boron distributions during extra corporal treatment of liver metastases by boron neutron capture therapy: a Monte Carlo simulation study.

    PubMed

    Khelifi, R; Nievaart, V A; Bode, P; Moss, R L; Krijger, G C

    2009-07-01

    A Monte Carlo calculation was carried out for boron neutron capture therapy (BNCT) of extra corporal liver phantom. The present paper describes the basis for a subsequent clinical application of the prompt gamma spectroscopy set-up aimed at in vivo monitoring of boron distribution. MCNP code was used first to validate the homogeneity in thermal neutron field in the liver phantom and simulate the gamma ray detection system (collimator and detector) in the treatment room. The gamma ray of 478 keV emitted by boron in small specific region can be detected and a mathematical formalism was used for the tomography image reconstruction. PMID:19394243

  15. Neutron-induced gamma-ray production

    SciTech Connect

    Nelson, R.O.; Drake, D.M.; Haight, R.C.; Laymon, C.M.; Wender, S.A.; Young, P.G. ); Drosg, M.; Pavlik, A.; Vonach, H. . Inst. fuer Radiumforschung und Kernphysik); Larson, D.C. )

    1990-01-01

    High resolution Ge detectors coupled with the WNR high-intensity, high-energy, pulsed neutron source at LAMPF recently have been used to measure a variety of reactions including (n,xn) for 1 {le} x {le} 11, (n,n{alpha}), (n,np), etc. The reactions are identified by the known gamma-ray energies of prompt transitions between the low lying states in the final nuclei. With our spallation neutron source cross section data are obtained at all neutron energies from a few MeV to over 200 MeV. Applications of the data range from assisting the interpretation of the planned Mars Observer mission to map the elemental composition of the martian surface, to providing data for nuclear model verification and understanding reaction mechanisms. For example, a study of the Pb(n,xn) reactions for 2 {le} x {le} 11 populating the first excited states of the even Pb isotopes is underway. These data will be used to test preequilibrium and other reaction models. 9 refs., 5 figs.

  16. Performance test results of noninvasive characterization of Resource Conservation and Recovery Act surrogate waste by prompt gamma neutron activation analysis

    SciTech Connect

    Gehrke, R.J.; Streier, G.G.

    1997-03-01

    During FY-96, a performance test was carried out with funding from the Mixed Waste Focus Area (MWFA) of the Department of Energy (DOE) to determine the noninvasive elemental assay capabilities of commercial companies for Resource Conservation and Recovery Act (RCRA) metals present in 8-gal drums containing surrogate waste. Commercial companies were required to be experienced in the use of prompt gamma neutron activation analysis (PGNAA) techniques and to have a prototype assay system with which to conduct the test assays. Potential participants were identified through responses to a call for proposals advertised in the Commerce Business Daily and through personal contacts. Six companies were originally identified. Two of these six were willing and able to participate in the performance test, as described in the test plan, with some subsidizing from the DOE MWFA. The tests were conducted with surrogate sludge waste because (1) a large volume of this type of waste awaits final disposition and (2) sludge tends to be somewhat homogeneous. The surrogate concentrations of the above RCRA metals ranged from {approximately} 300 ppm to {approximately} 20,000 ppm. The lower limit was chosen as an estimate of the expected sensitivity of detection required by noninvasive, pretreatment elemental assay systems to be of value for operational and compliance purposes and to still be achievable with state-of-the-art methods of analysis. The upper limit of {approximately} 20,000 ppm was chosen because it is the opinion of the author that assay above this concentration level is within current state-of-the-art methods for most RCRA constituents. This report is organized into three parts: Part 1, Test Plan to Evaluate the Technical Status of Noninvasive Elemental Assay Techniques for Hazardous Waste; Part 2, Participants` Results; and Part 3, Evaluation of and Comments on Participants` Results.

  17. Development of a technique using MCNPX code for determination of nitrogen content of explosive materials using prompt gamma neutron activation analysis method

    NASA Astrophysics Data System (ADS)

    Nasrabadi, M. N.; Bakhshi, F.; Jalali, M.; Mohammadi, A.

    2011-12-01

    Nuclear-based explosive detection methods can detect explosives by identifying their elemental components, especially nitrogen. Thermal neutron capture reactions have been used for detecting prompt gamma 10.8 MeV following radioactive neutron capture by 14N nuclei. We aimed to study the feasibility of using field-portable prompt gamma neutron activation analysis (PGNAA) along with improved nuclear equipment to detect and identify explosives, illicit substances or landmines. A 252Cf radio-isotopic source was embedded in a cylinder made of high-density polyethylene (HDPE) and the cylinder was then placed in another cylindrical container filled with water. Measurements were performed on high nitrogen content compounds such as melamine (C3H6N6). Melamine powder in a HDPE bottle was placed underneath the vessel containing water and the neutron source. Gamma rays were detected using two NaI(Tl) crystals. The results were simulated with MCNP4c code calculations. The theoretical calculations and experimental measurements were in good agreement indicating that this method can be used for detection of explosives and illicit drugs.

  18. Validating the ENDF-B/VII{sup 235}U(n{sub th},f) prompt fission neutron spectrum using updated dosimetry cross sections (IRDFF)

    SciTech Connect

    Capote, R.; Zolotarev, K. I.; Pronyaev, V. G.; Trkov, A.

    2012-07-01

    The International Reactor Dosimetry File IRDF-2002 released in 2004 by the IAEA contains cross-section data and corresponding uncertainties for 66 dosimetry reactions. New cross-section evaluations have become available recently that re-define some of these dosimetry reactions for reactor applications including: 1) high fidelity evaluation work undertaken by one of the authors (KIZ); 2) evaluations from the ENDF/B-VII libraries that cover reactions within the International Evaluation of Neutron Cross-Section Standards; and 3) evaluations from JENDL-3.1 and JENDL-4 libraries. Overall, 37 new evaluations of dosimetry reactions have been assessed to determine whether they should be adopted to update and improve IRDF-2002. A new dosimetry library (International Reactor Dosimetry File for Fission and Fusion - IRDFF) was assembled based on new evaluations combined with selected IRDF-2002 evaluations. A grand-total of 74 dosimetry reactions are included into the IRDFF dosimetry library available at www-nds.iaea.org/IRDFFI. The assembled library was used to validate the {sup 235}U(n{sub th},f) ENDF-B/VII.0 prompt fission neutron spectrum. An excellent average C/E value of 1.002 +/- 0.02 is achieved for reactions with mean neutron energy of the integrated response (E50%) lower than 11 MeV. C/E data for reactions with E50%-response higher than 11 MeV decreases up to 0.8. We conclude that the ENDF-B/VII.0 {sup 235}U(n{sub th},f) prompt fission neutron spectrum from 1-11 MeV is validated within quoted uncertainties by available integral measurements in {sup 235}U(n{sub th},f) neutron field. Further investigations for high-threshold reactions are needed and new measurements of spectrum average cross sections for those reactions in the {sup 235}U(n{sub th},f) neutron field are recommended. (authors)

  19. Induced Pairing Interaction in Neutron Star Matter

    NASA Astrophysics Data System (ADS)

    Lombardo, U.; Schulze, H.-J.; Zuo, W.

    2013-01-01

    The three superfluid phases supposed to occur in neutron stars are reviewed in the framework of the generalized BCS theory with the induced interaction. The structure of neutron stars characterized by beta-stable asymmetric nuclear matter in equilibrium with the gravitational force discloses new aspects of the pairing mechanism. Some of them are discussed in this report, in particular the formation in dense matter of Cooper pairs in the presence of three-body forces and the interplay between repulsive and attractive polarization effects on isospin T = 1 Cooper pairs embedded into the neutron and proton environment. Quantitative estimates of the energy gaps are reported and their sensitivity to the medium effects, i.e., interaction and polarization, is explored.

  20. Neutron-neutron angular correlations in spontaneous and neutron-induced fission

    NASA Astrophysics Data System (ADS)

    Vogt, Ramona; Randrup, Jorgen

    2015-04-01

    For many years, the state of the art for treating fission in radiation transport codes has involved sampling from average distributions. However, such average fission models have limited interaction-by-interaction capabilities. Energy is not explicitly conserved and no correlations are available because all particles are emitted isotropically and independently. However, in a true fission event, the energies, momenta and multiplicities of emitted particles are correlated. Such correlations are interesting for many modern applications, including detecting small amounts of material and detector development. Event-by-event generation of complete fission events are particularly useful because it is possible to obtain the fission products as well as the prompt neutrons and photons emitted during the fission process, all with complete kinematic information. It is therefore possible to extract any desired correlation observables. Such codes, when included in broader Monte Carlo transport codes, like MCNP, can be made broadly available. We compare results from our fast event-by-event fission code FREYA (Fission Reaction Event Yield Algorithm) with available neutron-neutron angular correlation data and study the sensitivities of these observables to the model inputs. This work was done under the auspices of the US DOE by (RV) LLNL, Contract DE-AC52-07NA27344, and by (JR) LBNL, Contract DE-AC02-05CH11231. We acknowledge support of the Office of Defense Nuclear Nonproliferation Research and Development in DOE/NNSA.

  1. The feasibility of in vivo quantification of bone-gadolinium in humans by prompt gamma neutron activation analysis (PGNAA) following gadolinium-based contrast-enhanced MRI

    NASA Astrophysics Data System (ADS)

    Mostafaei, F.; McNeill, F. E.; Chettle, D. R.; Noseworthy, M. D.; Prestwich, W. V.

    2015-11-01

    The feasibility of using a 238Pu/Be-based in vivo prompt γ-ray neutron activation analysis (IVNAA) system, previously successfully used for measurements of muscle, for the detection of gadolinium (Gd) in bone was presented. Gd is extensively used in contrast agents in MR imaging. We present phantom measurement data for the measurement of Gd in the tibia. Gd has seven naturally occurring isotopes, of which two have extremely large neutron capture cross sections; 155Gd (14.8% natural abundance (NA), σ= 60,900 barns) and 157Gd (15.65% NA, σ= 254,000 barns). Our previous work focused on muscle but this only informs about the short term kinetics of Gd. We studied the possibility of measuring bone, as it may be a long term storage site for Gd. A human simulating bone phantom set was developed. The phantoms were doped with seven concentrations of Gd of concentrations 0.0, 25, 50, 75, 100, 120 and 150 ppm. Additional elements important for neutron activation analysis, Na, Cl and Ca, were also included to create an overall elemental composition consistent with Reference Man. The overall conclusion is that the potential application of this Pu-Be-based prompt in vivo NAA for the monitoring of the storage and retention of Gd in bone is not feasible.

  2. Measurement of Neutron Induced and Spontaneous Fission in Pu-242 at DANCE

    NASA Astrophysics Data System (ADS)

    Chyzh, Andrii; Wu, C. Y.; Henderson, R.; Couture, A.; Lee, H. Y.; Ullmann, J.; O'Donnell, J. M.; Jandel, M.; Haight, R. C.; Bredeweg, T. A.; Dance Collaboration

    2013-10-01

    Neutron capture and fission reactions are important in nuclear engineering and physics. DANCE (Detector for Advanced Neutron Capture Measurement, LANL) combined with PPAC (avalanche technique based fission tagging detector, LLNL) were used to study neutron induced and spontaneous fission in 242Pu. 2 measurements were performed in 2013. The first experiment was done without the incident neutron beam with the fission tagging ability to study γ-rays emitted in the spontaneous fission of 242Pu. The second one - with the neutron beam to measure both the neutron capture and fission reactions. This is the first direct measurement of prompt fission γ-rays in 242Pu. The γ-ray multiplicity, γ-ray energy, and total energy of γ-rays per fission in 242Pu will be presented. These distributions of the 242Pu spontaneous fission will be compared to those in the 241Pu neutron induced fission. This work was performed under the auspices of the US Department of Energy by Los Alamos National Laboratory under Contract DE-AC52-06NA25396 and Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  3. Neutron-induced defects in optical fibers

    NASA Astrophysics Data System (ADS)

    Rizzolo, S.; Morana, A.; Cannas, M.; Bauer, S.; Perisse, J.; Mace, J.-R.; Boscaino, R.; Boukenter, A.; Ouerdane, Y.; Nacir, B.; Girard, S.

    2014-10-01

    We present a study on 0.8 MeV neutron-induced defects up to fluences of 1017 n/cm2 in fluorine doped optical fibers by using electron paramagnetic resonance, optical absorption and confocal micro-luminescence techniques. Our results allow to address the microscopic mechanisms leading to the generation of Silica-related point-defects such as E', H(I), POR and NBOH Centers.

  4. Neutron-induced defects in optical fibers

    SciTech Connect

    Rizzolo, S.; Morana, A.; Boukenter, A.; Ouerdane, Y.; Girard, S.; Cannas, M.; Boscaino, R.; Bauer, S.; Perisse, J.; Mace, J-R.; Nacir, B.

    2014-10-21

    We present a study on 0.8 MeV neutron-induced defects up to fluences of 10{sup 17} n/cm{sup 2} in fluorine doped optical fibers by using electron paramagnetic resonance, optical absorption and confocal micro-luminescence techniques. Our results allow to address the microscopic mechanisms leading to the generation of Silica-related point-defects such as E', H(I), POR and NBOH Centers.

  5. Developments for neutron-induced fission at IGISOL-4

    NASA Astrophysics Data System (ADS)

    Gorelov, D.; Penttilä, H.; Al-Adili, A.; Eronen, T.; Hakala, J.; Jokinen, A.; Kankainen, A.; Kolhinen, V. S.; Koponen, J.; Lantz, M.; Mattera, A.; Moore, I. D.; Pohjalainen, I.; Pomp, S.; Rakopoulos, V.; Reinikainen, J.; Rinta-Antila, S.; Simutkin, V.; Solders, A.; Voss, A.; Äystö, J.

    2016-06-01

    At the IGISOL-4 facility, neutron-rich, medium mass nuclei have usually been produced via charged particle-induced fission of natural uranium and thorium. Neutron-induced fission is expected to have a higher production cross section of the most neutron-rich species. Development of a neutron source along with a new ion guide continues to be one of the major goals since the commissioning of IGISOL-4. Neutron intensities at different angles from a beryllium neutron source have been measured in an on-line experiment with a 30 MeV proton beam. Recently, the new ion guide coupled to the neutron source has been tested as well. Details of the neutron source and ion guide design together with preliminary results from the first neutron-induced fission experiment at IGISOL-4 are presented in this report.

  6. Distribution of Prompt Neutron Emission Probability for Fission Fragments in Spontaneous Fission of 252Cf and 244,248Cm

    NASA Astrophysics Data System (ADS)

    Vorobyev, A. S.; Dushin, V. N.; Hambsch, F.-J.; Jakovlev, V. A.; Kalinin, V. A.; Laptev, A. B.; Petrov, B. F.; Shcherbakov, O. A.

    2005-05-01

    Neutrons emitted in fission events were measured separately for each complementary fragment in correlation with fission fragment energies. Two high-efficiency Gd-loaded liquid scintillator tanks were used for neutron registration. Fission fragment energies were measured using a twin Frisch gridded ionization chamber with a pinhole collimator. The neutron multiplicity distributions were obtained for each value of the fission fragment mass and energy and corrected for neutron registration efficiency, background, and pile-up. The dependency of these distributions on fragment mass and energy for different energy and mass bins as well as mass and energy distribution of fission fragments are presented and discussed.

  7. Intercomparison of inductively coupled plasma mass spectrometry, quantitative neutron capture radiography, and prompt gamma activation analysis for the determination of boron in biological samples.

    PubMed

    Schütz, C L; Brochhausen, C; Hampel, G; Iffland, D; Kuczewski, B; Otto, G; Schmitz, T; Stieghorst, C; Kratz, J V

    2012-10-01

    Boron determination in blood and tissue samples is a crucial task especially for treatment planning, preclinical research, and clinical application of boron neutron capture therapy (BNCT). Comparison of clinical findings remains difficult due to a variety of analytical methods, protocols, and standard reference materials in use. This paper addresses the comparability of inductively coupled plasma mass spectrometry, quantitative neutron capture radiography, and prompt gamma activation analysis for the determination of boron in biological samples. It was possible to demonstrate that three different methods relying on three different principles of sample preparation and boron detection can be validated against each other and yield consistent results for both blood and tissue samples. The samples were obtained during a clinical study for the application of BNCT for liver malignancies and therefore represent a realistic situation for boron analysis. PMID:22918535

  8. Ternary fission induced by polarized neutrons

    NASA Astrophysics Data System (ADS)

    Gönnenwein, Friedrich

    2013-12-01

    Ternary fission of (e,e) U- and Pu- isotopes induced by cold polarized neutrons discloses some new facets of the process. In the so-called ROT effect shifts in the angular distributions of ternary particles relative to the fission fragments show up. In the so-called TRI effect an asymmetry in the emission of ternary particles relative to a plane formed by the fragment momentum and the spin of the neutron appear. The two effects are shown to be linked to the components of angular momentum perpendicular and parallel to the fission axis at the saddle point of fission. Based on theoretical models the spectroscopic properties of the collective transitional states at the saddle point are inferred from experiment.

  9. Detailed Study of the Angular Correlations in the Prompt Neutron Emission in Spontaneous Fission of 252Cf

    NASA Astrophysics Data System (ADS)

    Kopatch, Yu.; Chietera, A.; Stuttgé, L.; Gönnenwein, F.; Mutterer, M.; Gagarski, A.; Guseva, I.; Chernysheva, E.; Dorvaux, O.; Hambsch, F.-J.; Hanappe, F.; Mezentseva, Z.; Telezhnikov, S.

    An experiment has been performed at IPHC Strasbourg, aimed at the detailed investigation of angular correlations in the neutron emission from spontaneous fission of 252Cf. Fission fragments were measured by the angle-sensitive double ionization chamber CODIS while neutrons were detected by a set of 60 DEMON scintillator counters. The main aim of the experiment is the observation of the correlation between the fragment spins and neutron emission anisotropy. Preliminary results, based on the Monte-Carlo simulations, as well as the preliminary analysis of the experimental data are shown.

  10. Neutron-induced peaks in Ge detectors from evaporation neutrons

    NASA Astrophysics Data System (ADS)

    Gete, E.; Measday, D. F.; Moftah, B. A.; Saliba, M. A.; Stocki, T. J.

    1997-02-01

    We have studied the peak shapes at 596 and 691 keV resulting from fast neutron interactions inside germanium detectors. We have used neutrons from a 252Cf source, as well as from the 28Si(μ -, nv), and 209Bi(π -, xn) reactions to compare the peaks and to check for a dependence of peak shape on the incoming neutron energy. In our investigation, no difference between these three measurements has been observed. In a comparison of these peak shapes with other studies, we found similar results to ours except for those measurements using monoenergetic neutrons in which a significant variation with neutron energy has been observed.

  11. Measurement of delayed-neutron yield from 237Np fission induced by thermal neutrons

    NASA Astrophysics Data System (ADS)

    Gundorin, N. A.; Zhdanova, K. V.; Zhuchko, V. E.; Pikelner, L. B.; Rebrova, N. V.; Salamatin, I. M.; Smirnov, V. I.; Furman, V. I.

    2007-06-01

    The delayed-neutron yield from thermal-neutron-induced fission of the 237Np nucleus was measured using a sample periodically exposed to a pulsed neutron beam with subsequent detection of neutrons during the time intervals between pulses. The experiment was realized on an Isomer-M setup mounted in the IBR-2 pulsed reactor channel equipped with a mirror neutron guide. The setup and the experimental procedure are described, the background sources are thoroughly analyzed, and the experimental data are presented. The total delayed-neutron yield from 237Np fission induced by thermal neutrons is ν d = 0.0110 ± 0.0009. This study was performed at the Frank Laboratory of Neutron Physics (JINR, Dubna).

  12. Prompt fission gamma-ray studies at DANCE

    SciTech Connect

    Jandel, M.; Rusev, G.; Bond, E. M.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M.. M; Haight, R. C.; Kawano, T.; Keksis, A. L.; Mosby, S. M.; O’Donnell, J. M.; Rundberg, R. S.; Stetcu, I.; Talou, P.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Stoyer, M. A.; Haslett, R. J.; Henderson, R. A.; Becker, J. A.; Wu, C. Y.

    2014-11-26

    Measurements of correlated data on prompt-fission γ-rays (PFG) have been carried out for various actinide isotopes in recent years using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory (LANL). We have developed a model that conveniently parametrizes the correlated data of γ-ray multiplicity and energy. New results on two- dimensional prompt-fission γ-ray multiplicity versus energy distributions from spontaneous fission on ²⁵²Cf and neutron-induced fission on 242mAm are presented together with previously obtained results on 233,235U and ²³⁹Pu. Correlated PFG data from ²⁵²Cf are also compared to results of the detailed theoretical model developed at LANL, for different thresholds of PFG energies. Future plans to measure correlated data on fission fragments, prompt fission neutrons and γ-rays at DANCE are presented.

  13. Measurement of the repeatability of the prompt flashlamp-induced wavefront aberration on beamlines at the National Ignition Facility

    NASA Astrophysics Data System (ADS)

    Homoelle, Doug; Bowers, Mark W.; Budge, Tracy; Haynam, Chris; Heebner, John; Hermann, Mark; Jancaitis, Ken; Jarboe, Jeff; Lafortune, Kai; Thaddeus Salmon, Joseph; Schindler, Tania; Shaw, Mike

    2011-08-01

    We have undertaken a measurement campaign to determine the repeatability of the prompt flashlamp-induced wavefront aberration on beamlines at the National Ignition Facility (NIF) and determine the extent to which shot-to-shot variations in this aberration may degrade the performance of a proposed adaptive optics system for the short-pulse Advanced Radiographic Capability beamline on NIF. In this paper we will describe the unique NIF configuration that was required to make this measurement, present the results of the experiment, and discuss the implications of these results for the adaptive optics system design.

  14. Neutron-induced single event burnout in high voltage electronics

    SciTech Connect

    Normand, E.; Wert, J.L.; Oberg, D.L.; Majewski, P.P.; Voss, P.; Wender, S.A.

    1997-12-01

    Energetic neutrons with an atmospheric neutron spectrum, which were demonstrated to induce single event burnout in power MOSFETs, have been shown to induce burnout in high voltage (>3,000V) electronics when operated at voltages as low as 50% of rated voltage. The laboratory failure rates correlate well with field failure rates measured in Europe.

  15. Monte Carlo simulation of prompt γ-ray spectra from depleted uranium under D-T neutron irradiation and electron recoil spectra in a liquid scintillator detector

    NASA Astrophysics Data System (ADS)

    Jian-Guo, Qin; Cai-Feng, Lai; Rong, Liu; Tong-Hua, Zhu; Xin-Wei, Zhang; Bang-Jiao, Ye

    2016-03-01

    To overcome the problem of inefficient computing time and unreliable results in MCNP5 calculation, a two-step method is adopted to calculate the energy deposition of prompt γ-rays in detectors for depleted uranium spherical shells under D-T neutron irradiation. In the first step, the γ-ray spectrum for energy below 7 MeV is calculated by MCNP5 code; secondly, the electron recoil spectrum in a BC501A liquid scintillator detector is simulated based on EGSnrc Monte Carlo Code with the γ-ray spectrum from the first step as input. The comparison of calculated results with experimental ones shows that the simulations agree well with experiment in the energy region 0.4-3 MeV for the prompt γ-ray spectrum and below 4 MeVee for the electron recoil spectrum. The reliability of the two-step method in this work is validated. Supported by the National Natural Science Foundation of China (91226104) and National Special Magnetic Confinement Fusion Energy Research, China (2015GB108001)

  16. Measurements of Prompt and MHD-Induced Fast Ion Loss from National Spherical Torus Experiment Plasmas

    SciTech Connect

    D.S. Darrow; S.S. Medley; A.L. Roquemore; W.W. Heidbrink; A. Alekseyev; F.E. Cecil; J. Egedal; V.Ya. Goloborod'ko; N.N. Gorelenkov; M. Isobe; S. Kaye; M. Miah; F. Paoletti; M.H. Redi; S.N. Reznik; A. Rosenberg; R. White; D. Wyatt; V.A. Yavorskij

    2002-10-15

    A range of effects may make fast ion confinement in spherical tokamaks worse than in conventional aspect ratio tokamaks. Data from neutron detectors, a neutral particle analyzer, and a fast ion loss diagnostic on the National Spherical Torus Experiment (NSTX) indicate that neutral beam ion confinement is consistent with classical expectations in quiescent plasmas, within the {approx}25% errors of measurement. However, fast ion confinement in NSTX is frequently affected by magnetohydrodynamic (MHD) activity, and the effect of MHD can be quite strong.

  17. Magnetic field induced differential neutron phase contrast imaging

    SciTech Connect

    Strobl, M.; Treimer, W.; Walter, P.; Keil, S.; Manke, I.

    2007-12-17

    Besides the attenuation of a neutron beam penetrating an object, induced phase changes have been utilized to provide contrast in neutron and x-ray imaging. In analogy to differential phase contrast imaging of bulk samples, the refraction of neutrons by magnetic fields yields image contrast. Here, it will be reported how double crystal setups can provide quantitative tomographic images of magnetic fields. The use of magnetic air prisms adequate to split the neutron spin states enables a distinction of field induced phase shifts and these introduced by interaction with matter.

  18. Yield of delayed neutrons in the thermal-neutron-induced reaction 245Cm( n, f)

    NASA Astrophysics Data System (ADS)

    Andrianov, V. R.; Vyachin, V. N.; Gundorin, N. A.; Druzhinin, A. A.; Zhdanova, K. V.; Lihachev, A. N.; Pikelner, L. B.; Rebrova, N. V.; Salamatin, I. M.; Furman, V. I.

    2008-10-01

    The yield of delayed neutrons, v d , from thermal-neutron-induced fission of 245Cm is measured. Experiments aimed at studying the properties of delayed neutrons from the fission of some reactor isotopes and initiated in 1997 were continued at the upgraded Isomer-M facility by a method according to which a periodic irradiation of a sample with a pulsed neutron beam from the IBR-2 reactor was accompanied by recording emitted neutrons in the intervals between the pulses. The accuracy of the resulting total delayed-neutron yield v d = (0.64 ± 0.02)% is two times higher than that in previous measurements. This work was performed at the Frank Laboratory of Neutron Physics at the Joint Institute for Nuclear Research (JINR, Dubna).

  19. Shape evolution in the neutron-rich osmium isotopes: Prompt γ-ray spectroscopy of Os196

    NASA Astrophysics Data System (ADS)

    John, P. R.; Modamio, V.; Valiente-Dobón, J. J.; Mengoni, D.; Lunardi, S.; Rodríguez, T. R.; Bazzacco, D.; Gadea, A.; Wheldon, C.; Alexander, T.; de Angelis, G.; Ashwood, N.; Barr, M.; Benzoni, G.; Birkenbach, B.; Bizzeti, P. G.; Bizzeti-Sona, A. M.; Bottoni, S.; Bowry, M.; Bracco, A.; Browne, F.; Bunce, M.; Camera, F.; Cederwall, B.; Corradi, L.; Crespi, F. C. L.; Désesquelles, P.; Eberth, J.; Farnea, E.; Fioretto, E.; Görgen, A.; Gottardo, A.; Grebosz, J.; Grente, L.; Hess, H.; Jungclaus, A.; Kokalova, Tz.; Korichi, A.; Korten, W.; Kuşoǧlu, A.; Lenzi, S.; Leoni, S.; Ljungvall, J.; Maron, G.; Meczynski, W.; Melon, B.; Menegazzo, R.; Michelagnoli, C.; Mijatović, T.; Million, B.; Molini, P.; Montagnoli, G.; Montanari, D.; Napoli, D. R.; Nolan, P.; Oziol, Ch.; Podolyák, Zs.; Pollarolo, G.; Pullia, A.; Quintana, B.; Recchia, F.; Reiter, P.; Roberts, O. J.; Rosso, D.; Şahin, E.; Salsac, M.-D.; Scarlassara, F.; Sferrazza, M.; Simpson, J.; Söderström, P.-A.; Stefanini, A. M.; Stezowski, O.; Szilner, S.; Theisen, Ch.; Ur, C. A.; Walshe, J.

    2014-08-01

    The shape transition in the neutron-rich Os isotopes is studied by investigating the neutron-rich 196Os nucleus through in-beam γ-ray spectroscopy using a two-proton transfer reaction from a 198Pt target to a 82Se beam. The beam-like recoils were detected and identified with the large-acceptance magnetic spectrometer PRISMA, and the coincident γ rays were measured with the advanced gamma tracking array (AGATA) demonstrator. The de-excitation of the low-lying levels of the yrast-band of 196Os were identified for the first time. The results are compared with state-of-the-art beyond-mean-field calculations, performed for the even-even 188-198Os isotopes. The new results suggest a smooth transition in the Os isotopes from a more axial rotational behavior towards predominately vibrational nuclei through triaxial configurations. An almost perfect γ-unstable/triaxial rotor yrast band is predicted for 196Os which is in agreement with the experimentally measured excited states.

  20. Neutron scattering studies in the actinide region. Progress report, August 1, 1992--July 31, 1993

    SciTech Connect

    Kegel, G.H.R.; Egan, J.J.

    1993-09-01

    This report discusses the following topics: Prompt fission neutron energy spectra for {sup 235}U and {sup 239}Pu; Two-parameter measurement of nuclear lifetimes; ``Black`` neutron detector; Data reduction techniques for neutron scattering experiments; Inelastic neutron scattering studies in {sup 197}Au; Elastic and inelastic scattering studies in {sup 239}Pu; and neutron induced defects in silicon dioxide MOS structures.

  1. Prompt repair of hydrogen peroxide-induced DNA lesions prevents catastrophic chromosomal fragmentation.

    PubMed

    Mahaseth, Tulip; Kuzminov, Andrei

    2016-05-01

    Iron-dependent oxidative DNA damage in vivo by hydrogen peroxide (H2O2, HP) induces copious single-strand(ss)-breaks and base modifications. HP also causes infrequent double-strand DNA breaks, whose relationship to the cell killing is unclear. Since hydrogen peroxide only fragments chromosomes in growing cells, these double-strand breaks were thought to represent replication forks collapsed at direct or excision ss-breaks and to be fully reparable. We have recently reported that hydrogen peroxide kills Escherichia coli by inducing catastrophic chromosome fragmentation, while cyanide (CN) potentiates both the killing and fragmentation. Remarkably, the extreme density of CN+HP-induced chromosomal double-strand breaks makes involvement of replication forks unlikely. Here we show that this massive fragmentation is further amplified by inactivation of ss-break repair or base-excision repair, suggesting that unrepaired primary DNA lesions are directly converted into double-strand breaks. Indeed, blocking DNA replication lowers CN+HP-induced fragmentation only ∼2-fold, without affecting the survival. Once cyanide is removed, recombinational repair in E. coli can mend several double-strand breaks, but cannot mend ∼100 breaks spread over the entire chromosome. Therefore, double-strand breaks induced by oxidative damage happen at the sites of unrepaired primary one-strand DNA lesions, are independent of replication and are highly lethal, supporting the model of clustered ss-breaks at the sites of stable DNA-iron complexes. PMID:27078578

  2. Evaluation of an in vivo prompt gamma neutron activation facility for body composition studies in critically ill intensive care patients: results on 41 normals

    SciTech Connect

    Beddoe, A.H.; Streat, S.J.; Hill, G.L.

    1984-03-01

    A programme of metabolic and nutritional research is being undertaken in critically ill patients requiring intensive care. Central to this research is the measurement of the three nutritionally important compartments of body composition, protein, fat, and water by a combination of tritium dilution and prompt gamma in vivo neutron activation analysis (IVNAA). In this paper a calibration technique is presented that enables absolute estimates of total body nitrogen (TBN) to be made using prompt gamma IVNAA in critically ill patients with gross abnormalities in body composition, especially in their state of hydration. This technique, which is independent of skinfold anthropometry and does not make a priori assumptions about the ratios of major body compartments, has been applied to 41 normal volunteers and the derived values for nitrogen compared with values obtained by applying three currently used calibration methods to the same experimental data. The empirical equations relate TBN in normal people to age, height, weight and sex. The mean ratios of experimental to predicted TBN (with SEMs) are 1.013 +/- 0.017 and 1.002 +/- 0.014, respectively. Mean values of the ratio of TBN to fat-free mass (0.0340 +/- 0.0004) and of total body water to fat-free mass (0.716 +/- 0.002) agree closely with values reported elsewhere for normals by a variety of techniques including chemical analysis. Finally, TBN results based on the four different calibration methods are presented for five surgical patients, demonstrating the importance of the calibration method on estimates of TBN in patients with abnormal body composition. It is concluded that this technique will provide accurate estimates of the total body content of protein, water, and fat in intensive care patients.

  3. Neutrons in cancer therapy

    NASA Astrophysics Data System (ADS)

    Allen, Barry J.

    1995-03-01

    The role of neutrons in the management of cancer has a long history. However, it is only in recent years that neutrons are beginning to find an accepted place as an efficacious radiation modality. Fast neutron therapy is already well established for the treatment of certain cancers, and clinical trials are ongoing. Californium neutron sources are being used in brachytherapy. Boron neutron capture therapy has been well tested with thermal neutrons and epithermal neutron dose escalation studies are about to commence in the USA and Europe. Possibilities of neutron induced auger electron therapy are also discussed. With respect to chemotherapy, prompt neutron capture analysis is being used to study the dose optimization of chemotherapy in the management of breast cancer. The rationales behind these applications of neutrons in the management of cancer are examined.

  4. Prompt Fission γ-ray Spectra Characteristics - A First Summary

    NASA Astrophysics Data System (ADS)

    Oberstedt, S.; Billnert, R.; Gatera, A.; Geerts, W.; Halipré, P.; Hambsch, F.-J.; Lebois, M.; Oberstedt, A.; Marini, P.; Vidali, M.; Wilson, J. N.

    In this work we give an overview of our investigations of prompt γ-ray emission in nuclear fission. This work was conducted during the last five years in response to a high priority nuclear data request formulated by the OECD/NEA. The aim was to reveal data deficiencies responsible for a severe under-prediction of the prompt γ heating in nuclear reactor cores. We obtained new prompt fission γ-ray spectral (PFGS) data for 252Cf(SF) as well as for thermal-neutron induced fission on 235U(nth,f) and 241Pu(nth,f). In addition, first PFGS measurements with a fast-neutron beam were accomplished, too. The impact of the new data and future data needs are discussed.

  5. An approach of reducing the background induced by neutrons

    NASA Technical Reports Server (NTRS)

    Shen, C.; Gu, Y.; Sun, Y.; Ma, Y.; Dai, C.; Fan, Z.

    1985-01-01

    The background induced by interactions of neutrons with detector material (and shield material) is difficult to be rejected. It is one of the most important factors to affect the sensitivity of a balloon-borne gamma-ray astronomical telescope. The main component of neutron flux at the major detector of the telescope is incident neutrons, that consists of atmospheric neutrons and neutrons locally produced in the balloon platform. Therefore, shielding the detector from incident neutrons is a possible way to reduce the background. NaI (T1) crystal is very widely used in gamma-ray astronomical telescopes. Through balloon-borne experiment it is shown that up 6 LiF shield is effective to reduce the background in NaI crystal.

  6. Pulsed neutron interrogation for detection of concealed special nuclear materials

    NASA Astrophysics Data System (ADS)

    Ruddy, Frank; Seidel, John; Flammang, Robert; Petrović, Bojan; Dulloo, Abdul; Congedo, Thomas

    2006-05-01

    A new neutron interrogation technique for detection of concealed Special Nuclear Material (SNM) is described. This technique is a combination of timing techniques from pulsed prompt gamma neutron activation analysis with silicon carbide (SiC) semiconductor fast neutron detector technology. SiC detectors are a new class of radiation detectors that are ultra-fast and capable of processing high count rates. SiC detectors can operate during and within nanoseconds of the end of an intense neutron pulse, providing the ability to detect the prompt neutron emissions from fission events produced by the neutrons in concealed SNM on a much faster pulsing time scale than has been achieved by other techniques. Neutron-induced fission neutrons in 235U have been observed in the time intervals between pulses of 14-MeV neutrons from a deuterium-tritium electronic neutron generator. Initial measurements have emphasized the detection of SNM using thermal-neutron induced fission. Neutron pulsing and time-sequenced neutron counts were carried out on a hundreds of microseconds time scale, enabling the observation of prompt fission neutrons induced by the die-away of thermal neutrons following the 14-MeV pulse. A discussion of pulsed prompt-neutron measurements and of SiC detectors as well as initial measurement results will be presented.

  7. Californium interrogation prompt neutron (CIPN) instrument for non-destructive assay of spent nuclear fuel-Design concept and experimental demonstration

    NASA Astrophysics Data System (ADS)

    Henzlova, D.; Menlove, H. O.; Rael, C. D.; Trellue, H. R.; Tobin, S. J.; Park, Se-Hwan; Oh, Jong-Myeong; Lee, Seung-Kyu; Ahn, Seong-Kyu; Kwon, In-Chan; Kim, Ho-Dong

    2016-01-01

    This paper presents results of the first experimental demonstration of the Californium Interrogation Prompt Neutron (CIPN) instrument developed within a multi-year effort launched by the Next Generation Safeguards Initiative Spent Fuel Project of the United States Department of Energy. The goals of this project focused on developing viable non-destructive assay techniques with capabilities to improve an independent verification of spent fuel assembly characteristics. For this purpose, the CIPN instrument combines active and passive neutron interrogation, along with passive gamma-ray measurements, to provide three independent observables. This paper describes the initial feasibility demonstration of the CIPN instrument, which involved measurements of four pressurized-water-reactor spent fuel assemblies with different levels of burnup and two initial enrichments. The measurements were performed at the Post-Irradiation Examination Facility at the Korea Atomic Energy Institute in the Republic of Korea. The key aim of the demonstration was to evaluate CIPN instrument performance under realistic deployment conditions, with the focus on a detailed assessment of systematic uncertainties that are best evaluated experimentally. The measurements revealed good positioning reproducibility, as well as a high degree of insensitivity of the CIPN instrument's response to irregularities in a radial burnup profile. Systematic uncertainty of individual CIPN instrument signals due to assembly rotation was found to be <4.5%, even for assemblies with fairly extreme gradients in the radial burnup profile. These features suggest that the CIPN instrument is capable of providing a good representation of assembly average characteristics, independent of assembly orientation in the instrument.

  8. Studies on fission with ALADIN. Precise and simultaneous measurement of fission yields, total kinetic energy and total prompt neutron multiplicity at GSI

    NASA Astrophysics Data System (ADS)

    Martin, Julie-Fiona; Taieb, Julien; Chatillon, Audrey; Bélier, Gilbert; Boutoux, Guillaume; Ebran, Adeline; Gorbinet, Thomas; Grente, Lucie; Laurent, Benoit; Pellereau, Eric; Alvarez-Pol, Héctor; Audouin, Laurent; Aumann, Thomas; Ayyad, Yassid; Benlliure, Jose; Casarejos, Enrique; Cortina Gil, Dolores; Caamaño, Manuel; Farget, Fanny; Fernández Domínguez, Beatriz; Heinz, Andreas; Jurado, Beatriz; Kelić-Heil, Aleksandra; Kurz, Nikolaus; Nociforo, Chiara; Paradela, Carlos; Pietri, Stéphane; Ramos, Diego; Rodríguez-Sànchez, Jose-Luis; Rodríguez-Tajes, Carme; Rossi, Dominic; Schmidt, Karl-Heinz; Simon, Haik; Tassan-Got, Laurent; Vargas, Jossitt; Voss, Bernd; Weick, Helmut

    2015-12-01

    A novel technique for fission studies, based on the inverse kinematics approach, is presented. Following pioneering work in the nineties, the SOFIA Collaboration has designed and built an experimental set-up dedicated to the simultaneous measurement of isotopic yields, total kinetic energies and total prompt neutron multiplicities, by fully identifying both fission fragments in coincidence, for the very first time. This experiment, performed at GSI, permits to study the fission of a wide variety of fissioning systems, ranging from mercury to neptunium, possibly far from the valley of stability. A first experiment, performed in 2012, has provided a large array of unprecedented data regarding the nuclear fission process. An excerpt of the results is presented. With this solid starter, further improvements of the experimental set-up are considered, which are consistent with the expected developments at the GSI facility, in order to measure more fission observables in coincidence. The completeness reached in the SOFIA data, permits to scrutinize the correlations between the interesting features of fission, offering a very detailed insight in this still unraveled mechanism.

  9. Mercury and gold concentrations of highly polluted environmental samples determined using prompt gamma-ray analysis and instrument neutron activation analysis

    NASA Astrophysics Data System (ADS)

    Osawa, Takahito; Hatsukawa, Yuichi; Appel, Peter W. U.; Matsue, Hideaki

    2011-04-01

    The authors have established a method of determining mercury and gold in severely polluted environmental samples using prompt gamma-ray analysis (PGA) and instrumental neutron activation analysis (INAA). Since large amounts of mercury are constantly being released into the environment by small-scale gold mining in many developing countries, the mercury concentration in tailings and water has to be determined to mitigate environmental pollution. Cold-vapor atomic absorption analysis, the most pervasive method of mercury analysis, is not suitable because tailings and water around mining facilities have extremely high mercury concentrations. On the other hand, PGA can determine high mercury concentrations in polluted samples as it has an appropriate level of sensitivity. Moreover, gold concentrations can be determined sequentially by using INAA after PGA. In conclusion, the analytical procedure established in this work using PGA and INAA is the best way to evaluate the degree of pollution and the tailing resource value. This method will significantly contribute to mitigating problems in the global environment.

  10. Neutron emission effects on fragment mass and kinetic energy distribution from fission of 239{sup Pu} induced by thermal neutrons

    SciTech Connect

    Montoya, M.; Rojas, J.; Lobato, I.

    2010-08-04

    The average of fragment kinetic energy (E-bar sign*) and the multiplicity of prompt neutrons ({nu}(bar sign)) as a function of fragment mass (m*), as well as the fragment mass yield (Y(m*)) from thermal neutron-induced fission of {sup 239}Pu have been measured by Tsuchiya et al.. In that work the mass and kinetic energy are calculated from the measured kinetic energy of one fragment and the difference of time of flight of the two complementary fragments. However they do not present their results about the standard deviation {sigma}{sub E}*(m*). In this work we have made a numerical simulation of that experiment which reproduces its results, assuming an initial distribution of the primary fragment kinetic energy (E(A)) with a constant value of the standard deviation as function of fragment mass ({sigma}{sub E}(A)). As a result of the simulation we obtain the dependence {sigma}{sub E}*(m*) which presents an enhancement between m* = 92 and m* = 110, and a peak at m* = 121.

  11. Low doses of neutrons induce changes in gene expression

    SciTech Connect

    Woloschak, G.E.; Chang-Liu, C.M. ); Panozzo, J.; Libertin, C.R. )

    1993-01-01

    Studies were designed to identify genes induced following low-dose neutron but not following [gamma]-ray exposure in fibroblasts. Our past work had shown differences in the expression of [beta]-protein kinase C and c-fos genes, both being induced following [gamma]-ray but not neutron exposure. We have identified two genes that are induced following neutron, but not [gamma]-ray, exposure: Rp-8 (a gene induced by apoptosis) and the long terminal repeat (LTR) of the human immunodeficiency (HIV). Rp-8 mRNA induction was demonstrated in Syrian hamster embryo fibroblasts and was found to be induced in cells exposed to neutrons administered at low (0.5 cGy/min) and at high dose rate (12 cGy/min). The induction of transcription from the LTR of HIV was demonstrated in HeLa cells bearing a transfected construct of the chloramphenicol acetyl transferase (CAT) gene driven by the HIV-LTR promoter. Measures of CAT activity and CAT transcripts following irradiation demonstrated an unresponsiveness to [gamma] rays over a broad range of doses. Twofold induction of the HIV-LTR was detected following neutron exposure (48 cGy) administered at low (0.5 cGy/min) but not high (12 cGy/min) dose rates. Ultraviolet-mediated HIV-LTR induction was inhibited by low-dose-rate neutron exposure.

  12. Low doses of neutrons induce changes in gene expression

    SciTech Connect

    Woloschak, G.E.; Chang-Liu, C.M.; Panozzo, J.; Libertin, C.R.

    1993-06-01

    Studies were designed to identify genes induced following low-dose neutron but not following {gamma}-ray exposure in fibroblasts. Our past work had shown differences in the expression of {beta}-protein kinase C and c-fos genes, both being induced following {gamma}-ray but not neutron exposure. We have identified two genes that are induced following neutron, but not {gamma}-ray, exposure: Rp-8 (a gene induced by apoptosis) and the long terminal repeat (LTR) of the human immunodeficiency (HIV). Rp-8 mRNA induction was demonstrated in Syrian hamster embryo fibroblasts and was found to be induced in cells exposed to neutrons administered at low (0.5 cGy/min) and at high dose rate (12 cGy/min). The induction of transcription from the LTR of HIV was demonstrated in HeLa cells bearing a transfected construct of the chloramphenicol acetyl transferase (CAT) gene driven by the HIV-LTR promoter. Measures of CAT activity and CAT transcripts following irradiation demonstrated an unresponsiveness to {gamma} rays over a broad range of doses. Twofold induction of the HIV-LTR was detected following neutron exposure (48 cGy) administered at low (0.5 cGy/min) but not high (12 cGy/min) dose rates. Ultraviolet-mediated HIV-LTR induction was inhibited by low-dose-rate neutron exposure.

  13. Neutron capture and neutron-induced fission experiments on americium isotopes with DANCE

    SciTech Connect

    Jandel, M.; Bredeweg, T. A.; Fowler, M. M.; Bond, E. M.; Couture, A.; Haight, R. C.; Keksis, A. L.; O'Donnell, J. M.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.; Stoyer, M. A.; Wu, C. Y.; Becker, J. A.; Haslett, R. J.; Henderson, R. A.

    2009-01-28

    Neutron capture cross section data on Am isotopes were measured using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory. The neutron capture cross section was determined for {sup 241}Am for neutron energies between thermal and 320 keV. Preliminary results were also obtained for {sup 243}Am for neutron energies between 10 eV and 250 keV. The results on concurrent neutron-induced fission and neutron-capture measurements on {sup 242m}Am will be presented where the fission events were actively triggered during the experiments. In these experiments, a Parallel-Plate Avalanche Counter (PPAC) detector that surrounds the target located in the center of the DANCE array was used as a fission-tagging detector to separate (n,{gamma}) events from (n,f) events. The first direct observation of neutron capture on {sup 242m}Am in the resonance region in between 2 and 9 eV of the neutron energy was obtained.

  14. Neutron capture and neutron-induced fission experiments on americium isotopes with DANCE

    SciTech Connect

    Jandel, Marian

    2008-01-01

    Neutron capture cross section data on Am isotopes were measured using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory. The neutron capture cross section was determined for {sup 241}Am for neutron energies between thermal and 320 keV. Preliminary results were also obtained for {sup 243}Am for neutron energies between 35 eV and 200 keV. The results on concurrent neutron-induced fission and neutron-capture measurements on {sup 242m}Am will be presented, where the fission events were actively triggered during the experiments. In these experiments, the Parallel-Plate Avalanche Counter (PPAC) detector that surrounds the target located in the center of the DANCE array was used as a fission-tagging detector to separate (n,{gamma}) from (n,f) events. The first evidence of neutron capture on {sup 242m}Am in the resonance region in between 2 and 9 eV of the neutron energy was obtained.

  15. Adiponectin exacerbates collagen-induced arthritis via enhancing Th17 response and prompting RANKL expression.

    PubMed

    Sun, Xiaoxuan; Feng, Xiaoke; Tan, Wenfeng; Lin, Na; Hua, Minhui; Wei, Yu; Wang, Fang; Li, Ningli; Zhang, Miaojia

    2015-01-01

    We previously reported adiponectin (AD) is highly expressed in the inflamed synovial joint tissue and correlates closely with progressive bone erosion in Rheumatoid arthritis (RA) patients. Here, we investigate the role of adiponectin in regulating Th17 response and the expression of receptor activator of nuclear factor-κB ligand (RANKL) in mice with CIA mice by intraarticularly injection of adiponectin into knee joints on day 17, day 20 and day 23 post first collagen immunization. The increased adiponectin expression was found in inflamed joint tissue of collagen-induced arthritis (CIA) mice. Adiponectin injection resulted in an earlier onset of arthritis, an aggravated arthritic progression, more severe synovial hyperplasia, bone erosion and osteoporosis in CIA mice. CD4(+)IL-17(+) Th17 cells, IL-17 mRNA and RANKL mRNA expression were markedly increased in the joint tissue of adiponectin treated CIA mice. Moreover, adiponectin treatment markedly enhanced Th17 cell generation from naive CD4(+) T cells in vitro, which accompanied by the high expression of Th17 transcription factor ROR-γt, and Th17 cytokine genes included IL-22 and IL-23. This study reveals a novel effect of adiponectin in exacerbating CIA progression by enhancing Th17 cell response and RANKL expression. PMID:26063682

  16. Actinide neutron-induced fission cross section measurements at LANSCE

    SciTech Connect

    Tovesson, Fredrik K; Laptev, Alexander B; Hill, Tony S

    2010-01-01

    Fission cross sections of a range of actinides have been measured at the Los Alamos Neutron Science Center (LANSCE) in support of nuclear energy applications in a wide energy range from sub-thermal energies up to 200 MeV. A parallel-plate ionization chamber are used to measure fission cross sections ratios relative to the {sup 235}U standard while incident neutron energies are determined using the time-of-flight method. Recent measurements include the {sup 233,238}U, {sup 239-242}Pu and {sup 243}Am neutron-induced fission cross sections. Obtained data are presented in comparison with ex isting evaluations and previous data.

  17. Neutron irradiation induced amorphization of silicon carbide

    SciTech Connect

    Snead, L.L.; Hay, J.C.

    1998-09-01

    This paper provides the first known observation of silicon carbide fully amorphized under neutron irradiation. Both high purity single crystal hcp and high purity, highly faulted (cubic) chemically vapor deposited (CVD) SiC were irradiated at approximately 60 C to a total fast neutron fluence of 2.6 {times} 10{sup 25} n/m{sup 2}. Amorphization was seen in both materials, as evidenced by TEM, electron diffraction, and x-ray diffraction techniques. Physical properties for the amorphized single crystal material are reported including large changes in density ({minus}10.8%), elastic modulus as measured using a nanoindentation technique ({minus}45%), hardness as measured by nanoindentation ({minus}45%), and standard Vickers hardness ({minus}24%). Similar property changes are observed for the critical temperature for amorphization at this neutron dose and flux, above which amorphization is not possible, is estimated to be greater than 130 C.

  18. Experimental study of some important characteristics of the thermal neutron induced fission of 237Np

    NASA Astrophysics Data System (ADS)

    Wagemans, C.; Allaert, E.; Caïtucoli, F.; D'hondt, P.; Barreau, G.; Perrin, P.

    1981-10-01

    Fission fragment mass and kinetic energy distributions and their correlations have been studied for the thermal neutron induced fission of 237Np. The global mass distribution is rather smooth, apart from a weak shoulder at μH = 140-141. When low excitation events are selected, fine structures associated with the charge of the fragments are observed. Furthermore, there is a sudden increase in Ek for μH > 155, which is probably due to a spherical shell N = 50 in the light fragment and the corresponding deformed (but stable) heavy fragments with masses in the rare earth region. For the average (pre-neutron emission) total fragment kinetic energy, a value of 176.4 ± 0.6 MeV has been obtained, in agreement with the systematics. Also the prompt neutron emission curve v(m ∗) has been calculated, which shows the well-known saw-tooth shape. Finally, the energy distribution and the emission probability of the ternary α-particles have been determined.

  19. Neutron-induced reaction studies using stored ions

    NASA Astrophysics Data System (ADS)

    Glorius, Jan; Litvinov, Yuri A.; Reifarth, René

    2015-11-01

    Storage rings provide unique possibilities for investigations of nuclear reactions. Radioactive ions can be stored if the ring is connected to an appropriate facility and reaction studies are feasible at low beam intensities because of the recycling of beam particles. Using gas jet or droplet targets, charged particle-induced reactions on short-lived isotopes can be studied in inverse kinematics. In such a system a high-flux reactor could serve as a neutron target extending the experimental spectrum to neutron-induced reactions. Those could be studied over a wide energy range covering the research fields of nuclear astrophysics and reactor safety, transmutation of nuclear waste and fusion.

  20. Total prompt γ-ray emission in fission

    NASA Astrophysics Data System (ADS)

    Wu, C. Y.; Chyzh, A.; Kwan, E.; Henserson, R. A.; Bredeweg, T. A.; Haight, R. C.; Hayes-Sterbenz, A. C.; Lee, H. Y.; O'Donnell, J. M.; Ullmann, J. L.

    2016-06-01

    The total prompt γ-ray energy distributions for the neutron-induced fission of 235U, 239,241Pu at incident neutron energy of 0.025 eV ‒ 100 keV, and the spontaneous fission of 252Cf were measured using the Detector for Advanced Neutron Capture Experiments (DANCE) array in coincidence with the detection of fission fragments by a parallel-plate avalanche counter. DANCE is a highly segmented, highly efficient 4π γ-ray calorimeter. Corrections were made to the measured distribution by unfolding the two-dimension spectrum of total γ-ray energy vs multiplicity using a simulated DANCE response matrix. The mean values of the total prompt γ-ray energy, determined from the unfolded distributions, are ~ 20% higher than those derived from measurements using single γ-ray detector for all the fissile nuclei studied. This raises serious concern on the validity of the mean total prompt γ-ray energy obtained from the product of mean values for both prompt γ-ray energy and multiplicity.

  1. Neutron-induced background in charge-coupled device detectors

    SciTech Connect

    Jaanimagi, P. A.; Boni, R.; Keck, R. L.

    2001-01-01

    The inertial confinement fusion (ICF) community must become more cognizant of the neutron-induced background levels in charge-coupled device (CCD) detectors that are replacing film as the recording medium in many ICF diagnostics. This background degrades the signal-to-noise ratio (SNR) of the recorded signals and for the highest-yield shots comprises a substantial fraction of the pixel's full well capacity. CCD detectors located anywhere in the OMEGA Target Bay are precluded from recording high precision signals (SNR>30) for deuterium--tritium neutron yields greater than 10{sup 13}. CCDs make excellent calibrated neutron detectors. The average CCD background level is proportional to the neutron yield, and we have measured a linear response over four decades. The spectrum of deposited energy per pixel is heavily weighted to low energies, <50 keV, with a few isolated saturated pixels. Most of the background recorded by the CCDs is due to secondary radiation produced by interactions of the primary neutrons with all the materials in the Target Bay as well as the shield walls and the floor. Since the noise source comes from all directions it is very difficult to shield. The fallback position of using film instead of CCD cameras for high-neutron-yield target shots is flawed, as we have observed substantially increased fog levels on our x-ray recording film as a function of the neutron yield.

  2. Neutron Induced Capture and Fission Processes on 238U

    NASA Astrophysics Data System (ADS)

    Oprea, Cristiana; Oprea, Alexandru

    2016-03-01

    Nuclear data on Uranium isotopes are of crucial interest for new generation of nuclear reactors. Processes of interest are the nuclear reactions induced by neutrons and in this work mainly the capture and the fission process on 238U will be analyzed in a wide energy interval. For slow and resonant neutrons the many levels Breit - Wigner formalism is necessary. In the case of fast and very fast neutrons up to 200 MeV the nuclear reaction mechanism implemented in Talys will be used. The present evaluations are necessary in order to obtain the field of neutrons in the design of nuclear reactors and they are compared with experimental data from literature obtained from capture and (n,xn) processes.

  3. Facility for neutron induced few body reactions at Bochum University

    NASA Astrophysics Data System (ADS)

    Bannach, B.; Bodek, K.; Börker, G.; Kamke, D.; Krug, J.; Lekkas, P.; Lübcke, W.; Stephan, M.

    1987-02-01

    A facility is described which is designed for the measurement of neutron induced three-body breakup. It has been used for the breakup of deuterium and of the nucleus 9Be. Neutrons are produced by a pulsed beam of deuterons from the Bochum 4MV Dynamitron-Tandem accelerator by bombarding a thick tritium-titanium target or a deuterium gas target. The outgoing beam is collimated by a 4π shielding to a solid angle of about 1 msr. In most cases, a liquid scintillator (NE232 or a mixture of NE232/NE213) serves as a target for the neutron beam. Scattered neutrons are detected by NE213-detectors of different sizes. For testing purposes the differential elastic n-d cross section and simultaneously the response of NE232 have been measured at 22.4 and 7.9 MeV.

  4. Basic Physics Data: Measurement of Neutron Multiplicity from Induced Fission

    SciTech Connect

    Pozzi, Sara; Haight, Robert

    2015-05-04

    From October 1 to October 17 a team of researchers from UM visited the LANSCE facility for an experiment during beam-time allotted from October 4 to October 17. A total of 24 detectors were used at LANSCE including liquid organic scintillation detectors (EJ-309), NaI scintillation detectors, and Li-6 enriched glass detectors. It is a double time-offlight (TOF) measurement using spallation neutrons generated by a target bombarded with pulsed high-energy protons. The neutrons travel to an LLNL-manufactured parallel plate avalanche chamber (PPAC) loaded with thin U-235 foils in which fission events are induced. The generated fission neutrons and photons are then detected in a detector array designed and built at UM and shipped to LANSCE. Preparations were made at UM, where setup and proposed detectors were tested. The UM equipment was then shipped to LANSCE for use at the 15L beam of the weapons neutron research (WNR) facility.

  5. Lanl Neutron-Induced Fission Cross Section Measurement Program

    NASA Astrophysics Data System (ADS)

    Laptev, A. B.; Tovesson, F.; Hill, T. S.

    2014-09-01

    A well established program of neutron-induced fission cross section measurement at Los Alamos Neutron Science Center (LANSCE) is supporting the Fuel Cycle Research program (FC R&D). Combining measurements at two LANSCE facilities, the Lujan Center and the Weapons Neutron Research facility (WNR), cover neutron energies over 10 orders of magnitude: from sub-thermal up to 200 MeV. A parallel-plate fission ionization chamber was used as a fission fragment detector. The 235U(n,f) standard was used as the reference. Fission cross sections have been measured for multiple actinides. The new data presented here completes the suite of long-lived Uranium isotopes that were investigated with this experimental approach. The cross section data are presented in comparison with existing evaluations and previous measurements.

  6. Neutron-induced defects in the lithium tetraborate single crystals

    NASA Astrophysics Data System (ADS)

    Burak, Y. V.; Padlyak, B. V.; Shevel, V. M.

    The X-band (nucongruent to9.4 GHz) electron spin resonance (ESR) spectra of the un-doped isotopically enriched lithium tetraborate (LTB) Li2B4O7 single crystals, irradiated by thermal neutrons (fluences Phi(n) =2.74x 10(15) divided by 1.79 x 10(18) cm(-2) ) were investigated at 300 and 77 K. The LTB crystals of high chemical purity and optical quality with different isotope compositions (Li-6(2) (B4O7)-B-10 , Li-6(2) (B4O7)-B-11 , Li-7(2) (B4O7)-B-10 and Li-7(2) (B4O7)-B-11) were grown by Czochralski technique. The thermal neutrons (the total quantity >90%) with fluence near 10(18) cm(-2) induce at least 4 different types of stable paramagnetic centers in the Li and B isotopically enriched LTB crystals. The ESR spectra, electron structure and efficiency of generation for centers, induced by thermal neutrons, essentially depend on neutron fluence and isotope composition of the LTB crystals. The local symmetry and the spin Hamiltonian parameters of the observed paramagnetic centers were determined and their electron structure were established. The possible models and formation mechanism of the radiation defects, induced by thermal neutrons in the LTB lattice, are proposed.

  7. Neutron-Induced Charged Particle Studies at LANSCE

    NASA Astrophysics Data System (ADS)

    Lee, Hye Young; Haight, Robert C.

    2014-09-01

    Direct measurements on neutron-induced charged particle reactions are of interest for nuclear astrophysics and applied nuclear energy. LANSCE (Los Alamos Neutron Science Center) produces neutrons in energy of thermal to several hundreds MeV. There has been an effort at LANSCE to upgrade neutron-induced charged particle detection technique, which follows on (n,z) measurements made previously here and will have improved capabilities including larger solid angles, higher efficiency, and better signal to background ratios. For studying cross sections of low-energy neutron induced alpha reactions, Frisch-gridded ionization chamber is designed with segmented anodes for improving signal-to-noise ratio near reaction thresholds. Since double-differential cross sections on (n,p) and (n,a) reactions up to tens of MeV provide important information on deducing nuclear level density, the ionization chamber will be coupled with silicon strip detectors (DSSD) in order to stop energetic charged particles. In this paper, we will present the status of this development including the progress on detector design, calibrations and Monte Carlo simulations. This work is funded by the US Department of Energy - Los Alamos National Security, LLC under Contract DE-AC52-06NA25396.

  8. Neutron induced fission of 234U

    NASA Astrophysics Data System (ADS)

    Hambsch, F.-J.; Al-Adili, A.; Oberstedt, S.; Pomp, S.

    2012-02-01

    The fission fragment properties of 234U(n,f) were investigated as a function of incident neutron energy from 0.2 MeV up to 5 MeV. The fission fragment mass, angular distribution and kinetic energy were measured with a double Frisch-grid ionization chamber using both analogue and digital data acquisition techniques. The reaction 234U(n,f) is relevant, since it involves the same compound nucleus as formed after neutron evaporation from highly excited 236U*, the so-called second-chance fission of 235U. Experimental data on fission fragment properties like fission fragment mass and total kinetic energy (TKE) as a function of incident neutron energy are rather scarce for this reaction. For the theoretical modelling of the reaction cross sections for Uranium isotopes this information is a crucial input parameter. In addition, 234U is also an important isotope in the Thorium-based fuel cycle. The strong anisotropy of the angular distribution around the vibrational resonance at En = 0.77 MeV could be confirmed using the full angular range. Fluctuations in the fragment TKE have been observed in the threshold region around the strong vibrational resonance at En = 0.77 MeV. The present results are in contradiction with corresponding literature values. Changes in the mass yield around the vibrational resonance and at En = 5 MeV relative to En = 2 MeV show a different signature. The drop in mean TKE around 2.5 to 3 MeV points to pair breaking as also observed in 235,238U(n,f). The measured two-dimensional mass yield and TKE distribution have been described in terms of fission modes. The yield of the standard 1 (S1) mode shows fluctuations in the threshold of the fission cross section due to the influence of the resonance and levels off at about 20% yield for higher incident neutron energies. The S2 mode shows the respective opposite behaviour. The mean TKE of both modes decreases with En. The decrease in mean TKE overrules the increase in S1 yield, so the mean TKE is dropping

  9. Cross sections of neutron-induced reactions

    SciTech Connect

    Mukhopadhyay, Tapan; Lahiri, Joydev; Basu, D. N.

    2010-10-15

    We study the properties of the neutron-nucleus total and reaction cross sections for several nuclei. We have applied an analytical model, the nuclear Ramsauer model, justified it from the nuclear reaction theory approach, and extracted the values of 12 parameters used in the model. The given parametrization has an advantage as phenomenological optical model potentials are limited up to 150-200 MeV. The present model provides good estimates of the total cross sections for several nuclei particularly at high energies.

  10. High Energy Neutron Induced Gamma Production

    SciTech Connect

    Brown, D A; Johnson, M; Navratil, P

    2007-09-28

    N Division has an interest in improving the physics and accuracy of the gamma data it provides to its customers. It was asked to look into major gamma producing reactions for 14 MeV incident neutrons for several low-Z materials and determine whether LLNL's processed data files faithfully represent the current state of experimental and theoretical knowledge for these reactions. To address this, we surveyed the evaluations of the requested materials, made recommendations for the next ENDL release and noted isotopes that will require further experimental study. This process uncovered several major problems in our translation and processing of the ENDF formatted evaluations, most of which have been resolved.

  11. Noise-induced dephasing in neutron interferometry

    SciTech Connect

    Sulyok, G.; Hasegawa, Y.; Rauch, H.; Klepp, J.; Lemmel, H.

    2010-05-15

    Decoherence phenomenona in a neutron interferometer are analyzed by simulation of the effects of an environment with magnetic noise fields. Basic calculations and experiments show the validity and limitations of this model system. In particular, loss and recovery of the interference pattern with controllable noise sources in both interferometer arms are discussed in detail. In addition, the decoherence behavior at high interference order, where Schroedinger-cat-like states exist in the interferometer, is investigated. While at low interference order a smearing of the interference pattern is observed, at high interference order a smearing of the modulated momentum distribution occurs.

  12. High-sensitivity transuranic waste assay by simultaneous proton and thermal-neutron interrogation using an electron linear accelerator

    SciTech Connect

    Franks, L.A.; Pigg, J.L.; Caldwell, J.T.; Cates, M.R.; Kunz, W.E.; Noel, B.W.

    1982-01-01

    Simultaneous photon and neutron interrogation from electron linear accelerator pulses is used as the basis for a unique assay technique for transuranics. Both prompt and delayed neutrons from the induced fissions are counted on a single detection system, and the contributions from each interrogating flux are resolved. Detection limits (3 sigma) for /sup 239/Pu were estimated to be 3 mg for prompt fission neutrons and 6 mg for delayed neutrons. The technique also provides a clear distinction between fissile and fertile nuclides.

  13. Imaging special nuclear material with muon-induced neutron emission.

    NASA Astrophysics Data System (ADS)

    Durham, J. Matthew

    2015-10-01

    Cosmic ray muons are a ubiquitous source of energetic charged particles that can be used to image high-Z material through significant amounts of shielding. Negative muons which come to rest inside fissile material can be captured into atomic orbitals and induce fission, which may lead to detectable neutron emission. Muon tracks that are correlated with neutron emission can therefore serve as a signal for the presence of fissile material, and laminography with the tagged muon tracks can be performed to produce an image of the neutron emission source. In this presentation, we will discuss results of imaging tests using this technique at Los Alamos National Laboratory, and possible applications in treaty verification.

  14. Neutrino Signal of Collapse-induced Thermonuclear Supernovae: The Case for Prompt Black Hole Formation in SN 1987A

    NASA Astrophysics Data System (ADS)

    Blum, Kfir; Kushnir, Doron

    2016-09-01

    Collapse-induced thermonuclear explosion (CITE) may explain core-collapse supernovae (CCSNe). We analyze the neutrino signal in CITE and compare it to the neutrino burst of SN 1987A. For strong (≳ {10}51 erg) CCSNe, such as SN 1987A, CITE predicts a proto-neutron star (PNS) accretion phase lasting up to a few seconds that is cut off by black hole (BH) formation. The neutrino luminosity can later be revived by accretion disk emission after a dead time of a few to a few tens of seconds. In contrast, the neutrino mechanism for CCSNe predicts a short (≲s) PNS accretion phase, followed by slowly declining PNS cooling luminosity. We repeat statistical analyses used in the literature to interpret the neutrino mechanism, and apply them to CITE. The first 1–2 s of the neutrino burst are equally compatible with CITE and with the neutrino mechanism. However, the data points toward a luminosity drop at t = 2–3 s, which is in some tension with the neutrino mechanism but can be naturally attributed to BH formation in CITE. The occurrence of neutrino signal events at 5 s suggests that, within CITE, the accretion disk formed by that time. We perform two-dimensional numerical simulations showing that CITE may be able to accommodate this disk formation time while reproducing the ejected 56Ni mass and ejecta kinetic energy within factors of 2–3 of observations. We estimate the accretion disk neutrino luminosity, finding it to be on the low side but compatible with the data to a factor of 10. Given comparable uncertainties in the disk luminosity simulation, we conclude that direct BH formation may have occurred in SN 1987A.

  15. Spatial corrections for pulsed-neutron reactivity measurements.

    SciTech Connect

    Cao, Y.; Lee, J.; Nuclear Engineering Division; Univ. of Michigan

    2010-07-01

    For pulsed-neutron experiments performed in a subcritical reactor, the reactivity obtained from the area-ratio method is sensitive to detector positions. The spatial effects are induced by the presence of both the prompt neutron harmonics and the delayed neutron harmonics in the reactor. The traditional kinetics distortion factor is only limited to correcting the spatial effects caused by the fundamental prompt-{alpha} mode. In this paper, we derive spatial correction factors fp and fd to account for spatial effects induced by the prompt neutron harmonics and the delayed neutron harmonics, respectively. Our numerical simulations with the FX2-TH time-dependent multigroup diffusion code indicate that the high-order prompt neutron harmonics lead to significant spatial effects and cannot be neglected in calculating the spatial correction factors. The prompt spatial correction factor fp can be simply determined by the ratio of the normalized detector responses corresponding to the fundamental k-mode and the prompt neutron flux integrated over the pulse period. Thus, it is convenient to calculate and provides physically intuitive explanations on the spatial dependence of reactivity measured in the MUSE-4 experiments: overestimation of the subcriticality in regions close to the external neutron source and underestimation of the subcriticality away from the source but within the fuel region.

  16. Prompt fission gamma-ray studies at DANCE

    DOE PAGESBeta

    Jandel, M.; Rusev, G.; Bond, E. M.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M.. M; Haight, R. C.; Kawano, T.; Keksis, A. L.; et al

    2014-11-26

    Measurements of correlated data on prompt-fission γ-rays (PFG) have been carried out for various actinide isotopes in recent years using the Detector for Advanced Neutron Capture Experiments (DANCE) at Los Alamos National Laboratory (LANL). We have developed a model that conveniently parametrizes the correlated data of γ-ray multiplicity and energy. New results on two- dimensional prompt-fission γ-ray multiplicity versus energy distributions from spontaneous fission on ²⁵²Cf and neutron-induced fission on 242mAm are presented together with previously obtained results on 233,235U and ²³⁹Pu. Correlated PFG data from ²⁵²Cf are also compared to results of the detailed theoretical model developed at LANL,more » for different thresholds of PFG energies. Future plans to measure correlated data on fission fragments, prompt fission neutrons and γ-rays at DANCE are presented.« less

  17. Dependence of Delayed-Neutron Energy Spectra on the Energy of Neutrons which Induce Fission of Uranium -235

    NASA Astrophysics Data System (ADS)

    Sharfuddin, Quazi

    Delayed neutron energy spectra following both fast and thermal neutron induced fission of U-235 are measured by the time-of-flight technique using beta-neutron correlations. Fast neutrons are produced via the (p,n) reaction in Li-7 using the University of Lowell 5.5 MV Van de Graaff Accelerator, whereas thermal neutrons are produced by surrounding the fission chamber and target assembly with paraffin. Fission fragments stopped in the helium atmosphere of the fission chamber are transferred by a helium jet system to a low background counting room where the composite delayed neutron energy spectra are measured as a function of time after fission. The delayed neutron energy spectra following fast fission of U-235 are compared to those resulting from thermal fission of U-235. Two mathematical methods are developed to deduce the equilibrium delayed neutron spectrum from the composite delayed neutron spectra measured as a function of delay time after fission. These methods are then applied to obtain the equilibrium delayed neutron spectrum from thermal fission of U-235. Finally, the six-group delayed neutron spectra resulting from thermal fission of U-235 are deduced from the measured composite delayed neutron spectra as a function of delay time after fission using a matrix inversion method.

  18. Genotoxicity of neutrons in Drosophila melanogaster. Somatic mutation and recombination induced by reactor neutrons.

    PubMed

    Guzmán-Rincón, J; Delfín-Loya, A; Ureña-Núñez, F; Paredes, L C; Zambrano-Achirica, F; Graf, U

    2005-08-01

    This paper describes the observation of a direct relationship between the absorbed doses of neutrons and the frequencies of somatic mutation and recombination using the wing somatic mutation and recombination test (SMART) of Drosophila melanogaster. This test was used for evaluating the biological effects induced by neutrons from the Triga Mark III reactor of Mexico. Two different reactor power levels were used, 300 and 1000 kW, and two absorbed doses were tested for each power level: 1.6 and 3.2 Gy for 300 kW and 0.84 and 1.7 Gy for 1000 kW. A linear relationship was observed between the absorbed dose and the somatic mutation and recombination frequencies. Furthermore, these frequencies were dependent on larval age: In 96-h-old larvae, the frequencies were increased considerably but the sizes of the spots were smaller than in 72-h-old larvae. The analysis of the balancer-heterozygous progeny showed a linear absorbed dose- response relationship, although the responses were clearly lower than found in the marker-trans-heterozygous flies. Approximately 65% of the genotoxicity observed is due to recombinational events. The results of the study indicate that thermal and fast neutrons are both mutagenic and recombinagenic in the D. melanogaster wing SMART, and that the frequencies are dependent on neutron dose, reactor power, and the age of the treated larvae. PMID:16038586

  19. Detecting special nuclear material using muon-induced neutron emission

    NASA Astrophysics Data System (ADS)

    Guardincerri, Elena; Bacon, Jeffrey; Borozdin, Konstantin; Matthew Durham, J.; Fabritius, Joseph, II; Hecht, Adam; Milner, Edward C.; Miyadera, Haruo; Morris, Christopher L.; Perry, John; Poulson, Daniel

    2015-07-01

    The penetrating ability of cosmic ray muons makes them an attractive probe for imaging dense materials. Here, we describe experimental results from a new technique that uses neutrons generated by cosmic-ray muons to identify the presence of special nuclear material (SNM). Neutrons emitted from SNM are used to tag muon-induced fission events in actinides and laminography is used to form images of the stopping material. This technique allows the imaging of SNM-bearing objects tagged using muon tracking detectors located above or to the side of the objects, and may have potential applications in warhead verification scenarios. During the experiment described here we did not attempt to distinguish the type or grade of the SNM.

  20. Evaluation of photon production data from neutron-induced reactions

    SciTech Connect

    Fu, C.Y.

    1980-01-01

    The evaluation methods and procedures used for generating the photon production data in the current Evaluated Nuclear Data File (ENDF/B, Version V) are reviewed. There are 42 materials in the General Purpose File of ENDF/B-V that contain data for prompt photon production. Almost all evaluations had substantial experimental data bases, but fewer than half of them employed any of the following evaluation methods. Only a few used theoretical techniques that are sophisticated enough to ensure internal consistency with other particle production data. Comments are made on four evaluation methods: the empirical formalism of Howerton et al., the Troubetzkoy model, the multiparticle Hauser-Feshbach/precompound model, and the Yost method. Critiques are also made on three procedures used for conserving photon energies in neutron capture reactions. The presence of photon production data in the file is useful for studying energy balance, since photon production generally accounts for a large portion of the reaction energy output. Problems found in energy balance checks are discussed. 9 figures, 1 table.

  1. Muon-Induced Neutrons Do Not Explain the DAMA Data

    NASA Astrophysics Data System (ADS)

    Klinger, J.; Kudryavtsev, V. A.

    2015-04-01

    We present an accurate model of the muon-induced background in the DAMA/LIBRA experiment. Our work challenges proposed mechanisms which seek to explain the observed DAMA signal modulation with muon-induced backgrounds. Muon generation and transport are performed using the MUSIC /MUSUN code, and subsequent interactions in the vicinity of the DAMA detector cavern are simulated with Geant4. We estimate the total muon-induced neutron flux in the detector cavern to be Φnν=1.0 ×10-9 cm-2 s-1 . We predict 3.49 ×10-5 counts /day /kg /keV , which accounts for less than 0.3% of the DAMA signal modulation amplitude.

  2. Muon-Induced Neutrons Do Not Explain the DAMA Data.

    PubMed

    Klinger, J; Kudryavtsev, V A

    2015-04-17

    We present an accurate model of the muon-induced background in the DAMA/LIBRA experiment. Our work challenges proposed mechanisms which seek to explain the observed DAMA signal modulation with muon-induced backgrounds. Muon generation and transport are performed using the MUSIC/MUSUN code, and subsequent interactions in the vicinity of the DAMA detector cavern are simulated with Geant4. We estimate the total muon-induced neutron flux in the detector cavern to be Φ(n)(ν)=1.0 × 10(-9)  cm(-2) s(-1). We predict 3.49 × 10(-5)  counts/day/kg/keV, which accounts for less than 0.3% of the DAMA signal modulation amplitude. PMID:25933303

  3. Fission of Actinides Induced by Neutrons at nTOF

    SciTech Connect

    Tassan-Got, L.; Audouin, L.; Berthier, B.; Ferrant, L.; Isaev, S.; Le Naour, C.; Stephan, C.; Trubert, D.; Duran, I.; Paradela, C.; Moreau, C.

    2005-05-24

    The neutron-induced fission cross sections of 233U, 234U, 232Th, 237Np, 209Bi, natPb have been measured on the nTOF facility at CERN, which allows an accurate energy measurement owing to the long path. Parallel plate avalanche counters were used to detect the 2 fission fragments in coincidence. This method allows an efficient discrimination of fission reactions among other types of reactions especially at high energies, and it is well suited for the very large energy range available at nTOF. The case of 234U will be used as an example of the quality of the data obtained in these measurements.

  4. Neutron distribution and induced activity inside a Linac treatment room.

    PubMed

    Juste, B; Miró, R; Verdú, G; Díez, S; Campayo, J M

    2015-08-01

    Induced radioactivity and photoneutron contamination inside a radiation therapy bunker of a medical linear accelerator (Linac) is investigated in this work. The Linac studied is an Elekta Precise electron accelerator which maximum treatment photon energy is 15 MeV. This energy exceeds the photonuclear reaction threshold (around 7 MeV for high atomic number metals). The Monte Carlo code MCNP6 has been used for quantifying the neutron contamination inside the treatment room for different gantry rotation configuration. Walls activation processes have also been simulated. The approach described in this paper is useful to prevent the overexposure of patients and medical staff. PMID:26737878

  5. Neutron-induced reaction studies at FIGARO using a spallation source

    NASA Astrophysics Data System (ADS)

    Rochman, D.; Haight, R. C.; O'Donnell, J. M.; Devlin, M.; Ethvignot, T.; Granier, T.

    2004-05-01

    A description is given of the new flexible facility Fast Neutron-Induced Gamma-Ray Observer (FIGARO) at the Los Alamos Neutron Science Center. FIGARO is designed to study fast-neutron-induced reactions that result in the emission of γ rays and neutrons, using the white neutron beam of the Weapons Neutron Research Facility. The emitted neutrons and γ rays are detected by several liquid scintillators and one high-resolution germanium or one barium-fluoride detector, respectively. As an example, the inelastic neutron scattering on Si from 4 to 20 MeV is presented and the results are compared with predictions of the nuclear model calculations performed with the codes GNASH and EMPIRE II.

  6. The Upgrade of the Neutron Induced Positron Source NEPOMUC

    NASA Astrophysics Data System (ADS)

    Hugenschmidt, C.; Ceeh, H.; Gigl, T.; Lippert, F.; Piochacz, C.; Pikart, P.; Reiner, M.; Weber, J.; Zimnik, S.

    2013-06-01

    In summer 2012, the new NEutron induced POsitron Source MUniCh (NEPOMUC) was installed and put into operation at the research reactor FRM II. At NEPOMUC upgrade 80% 113Cd enriched Cd is used as neutron-gamma converter in order to ensure an operation time of 25 years. A structure of Pt foils inside the beam tube generates positrons by pair production. Moderated positrons leaving the Pt front foil are electrically extracted and magnetically guided to the outside of the reactor pool. The whole design, including Pt-foils, the electric lenses and the magnetic fields, has been improved in order to enhance both the intensity and the brightness of the positron beam. After adjusting the potentials and the magnetic guide and compensation fields an intensity of about 3·109 moderated positrons per second is expected. During the first start-up, the measured temperatures of about 90°C ensure a reliable operation of the positron source. Within this contribution the features and the status of NEPOMUC upgrade are elucidated. In addition, an overview of recent positron beam experiments and current developments at the spectrometers is given.

  7. Evaluation of proton inelastic reaction models in Geant4 for prompt gamma production during proton radiotherapy

    NASA Astrophysics Data System (ADS)

    Jeyasugiththan, Jeyasingam; Peterson, Stephen W.

    2015-10-01

    During proton beam radiotherapy, discrete secondary prompt gamma rays are induced by inelastic nuclear reactions between protons and nuclei in the human body. In recent years, the Geant4 Monte Carlo toolkit has played an important role in the development of a device for real time dose range verification purposes using prompt gamma radiation. Unfortunately the default physics models in Geant4 do not reliably replicate the measured prompt gamma emission. Determining a suitable physics model for low energy proton inelastic interactions will boost the accuracy of prompt gamma simulations. Among the built-in physics models, we found that the precompound model with a modified initial exciton state of 2 (1 particle, 1 hole) produced more accurate discrete gamma lines from the most important elements found within the body such as 16O, 12C and 14N when comparing them with the available gamma production cross section data. Using the modified physics model, we investigated the prompt gamma spectra produced in a water phantom by a 200 MeV pencil beam of protons. The spectra were attained using a LaBr3 detector with a time-of-flight (TOF) window and BGO active shield to reduce the secondary neutron and gamma background. The simulations show that a 2 ns TOF window could reduce 99% of the secondary neutron flux hitting the detector. The results show that using both timing and active shielding can remove up to 85% of the background radiation which includes a 33% reduction by BGO subtraction.

  8. Evaluation of proton inelastic reaction models in Geant4 for prompt gamma production during proton radiotherapy.

    PubMed

    Jeyasugiththan, Jeyasingam; Peterson, Stephen W

    2015-10-01

    During proton beam radiotherapy, discrete secondary prompt gamma rays are induced by inelastic nuclear reactions between protons and nuclei in the human body. In recent years, the Geant4 Monte Carlo toolkit has played an important role in the development of a device for real time dose range verification purposes using prompt gamma radiation. Unfortunately the default physics models in Geant4 do not reliably replicate the measured prompt gamma emission. Determining a suitable physics model for low energy proton inelastic interactions will boost the accuracy of prompt gamma simulations. Among the built-in physics models, we found that the precompound model with a modified initial exciton state of 2 (1 particle, 1 hole) produced more accurate discrete gamma lines from the most important elements found within the body such as 16O, 12C and 14N when comparing them with the available gamma production cross section data. Using the modified physics model, we investigated the prompt gamma spectra produced in a water phantom by a 200 MeV pencil beam of protons. The spectra were attained using a LaBr3 detector with a time-of-flight (TOF) window and BGO active shield to reduce the secondary neutron and gamma background. The simulations show that a 2 ns TOF window could reduce 99% of the secondary neutron flux hitting the detector. The results show that using both timing and active shielding can remove up to 85% of the background radiation which includes a 33% reduction by BGO subtraction. PMID:26389549

  9. α and 2 p 2 n emission in fast neutron-induced reactions on 60Ni

    NASA Astrophysics Data System (ADS)

    Fotiades, N.; Devlin, M.; Haight, R. C.; Nelson, R. O.; Kunieda, S.; Kawano, T.

    2015-06-01

    Background: The cross sections for populating the residual nucleus in the reaction ZAX(n,x) Z -2 A -4Y exhibit peaks as a function of incident neutron energy corresponding to the (n ,n'α ) reaction and, at higher energy, to the (n ,2 p 3 n ) reaction. The relative magnitudes of these peaks vary with the Z of the target nucleus. Purpose: Study fast neutron-induced reactions on 60Ni. Locate experimentally the nuclear charge region along the line of stability where the cross sections for α emission and for 2 p 2 n emission in fast neutron-induced reactions are comparable as a further test of reaction models. Methods: Data were taken by using the Germanium Array for Neutron-Induced Excitations. The broad-spectrum pulsed neutron beam of the Los Alamos Neutron Science Center's Weapons Neutron Research facility provided neutrons in the energy range from 1 to 250 MeV. The time-of-flight technique was used to determine the incident-neutron energies. Results: Absolute partial cross sections for production of seven discrete Fe γ rays populated in 60Ni (n ,α /2 p x n γ ) reactions with 2 ≤x ≤5 were measured for neutron energies 1 MeVneutron energies while discrepancies appear at higher neutron energies. The cross section for producing an isotope in fast neutron-induced reactions on stable targets via α emission at the peak of the (n ,α ) and (n ,n'α ) reactions is comparable to that for 2 p 2 n and 2 p 3 n emission at higher incident energies in the nuclear charge region around Fe.

  10. Dependence on neutron energy of neutron-induced peaks in Ge detectors

    NASA Astrophysics Data System (ADS)

    Gete, E.; Measday, David F.; Moftah, B. A.; Saliba, M. A.; Stocki, Trevor J.

    1997-02-01

    We have studied the peak shapes at 596 and 691 KeV resulting from fast neutron interactions inside germanium detectors. We have used neutrons from a 252Cf source, as well as from the 28Si((mu) -, nv), and 209Bi((pi) -, xn) reactions to compare the peaks and to check for any dependence of peak shape on the incoming neutron energy. In our investigation, no dependence of these peak shapes on the neutron energy spectra has been observed. In a comparison of these peak shapes with other studies we found similar results to ours except for monoenergetic neutron irradiations from 1 to 8 MeV.

  11. SU-E-J-100: Reconstruction of Prompt Gamma Ray Three Dimensional SPECT Image From Boron Neutron Capture Therapy(BNCT)

    SciTech Connect

    Yoon, D; Jung, J; Suh, T

    2014-06-01

    Purpose: Purpose of paper is to confirm the feasibility of acquisition of three dimensional single photon emission computed tomography (SPECT) image from boron neutron capture therapy (BNCT) using Monte Carlo simulation. Methods: In case of simulation, the pixelated SPECT detector, collimator and phantom were simulated using Monte Carlo n particle extended (MCNPX) simulation tool. A thermal neutron source (<1 eV) was used to react with the boron uptake region (BUR) in the phantom. Each geometry had a spherical pattern, and three different BURs (A, B and C region, density: 2.08 g/cm3) were located in the middle of the brain phantom. The data from 128 projections for each sorting process were used to achieve image reconstruction. The ordered subset expectation maximization (OSEM) reconstruction algorithm was used to obtain a tomographic image with eight subsets and five iterations. The receiver operating characteristic (ROC) curve analysis was used to evaluate the geometric accuracy of reconstructed image. Results: The OSEM image was compared with the original phantom pattern image. The area under the curve (AUC) was calculated as the gross area under each ROC curve. The three calculated AUC values were 0.738 (A region), 0.623 (B region), and 0.817 (C region). The differences between length of centers of two boron regions and distance of maximum count points were 0.3 cm, 1.6 cm and 1.4 cm. Conclusion: The possibility of extracting a 3D BNCT SPECT image was confirmed using the Monte Carlo simulation and OSEM algorithm. The prospects for obtaining an actual BNCT SPECT image were estimated from the quality of the simulated image and the simulation conditions. When multiple tumor region should be treated using the BNCT, a reasonable model to determine how many useful images can be obtained from the SPECT could be provided to the BNCT facilities. This research was supported by the Leading Foreign Research Institute Recruitment Program through the National Research

  12. Experimental Evaluation of Neutron Induced Noise on Gated X-ray Framing Cameras

    SciTech Connect

    Izumi, N; Stone, G; Hagmann, C; Sorce, C; Bradley, D K; Moran, M; Landen, O L; Stoeffl, W; Springer, P; Tommasini, R; Hermann, H W; Kyrala, G A; Glebov, V Y; Sangster, T C; Koch, J A

    2009-10-08

    A micro-channel plate based temporally-gated x-ray camera (framing camera) is one of the most versatile diagnostic tools of inertial confinement fusion experiments; particularly for observation of the shape of x-ray self emission from compressed core of imploded capsules. However, components used in an x-ray framing camera have sensitivity to neutrons induced secondary radiations. On early low-yield capsule implosions at the National Ignition Facility (NIF), the expected neutron production is about 5 x 10{sup 14}. Therefore, the expected neutron fluence at a framing camera located {approx} 150 cm from the object is 2 x 10{sup 9} neutrons/cm{sup 2}. To obtain gated x-ray images in such harsh neutron environments, quantitative understanding of neutron-induced backgrounds is crucial.

  13. Explosive Material Identification via Neutron-Induced Gamma Rays

    NASA Astrophysics Data System (ADS)

    Freiberg, David; Litz, Marc

    2014-09-01

    With the increase in the usage of improvised explosive devices, both vehicle-borne and buried, it has become increasingly important to quickly identify potentially explosive materials before they can be detonated. In a field test performed in January of 2014, 14 MeV neutrons generated in a deuterium-tritium reaction induced gamma emissions in explosive material targets. The resulting gamma rays were counted in LaBr3 detectors in both a time-binned associated particle imaging (API) mode and a repetitively pulsed mode. The details of the resulting data sets were analyzed, and gamma lines for carbon, oxygen, and nitrogen were identified in the spectra produced by both modes. Post-test noise reduction techniques included empty hole background subtraction, Compton background subtraction, peak area integration, and time-of-flight gating. The induced C, O, and N gamma line intensities and ratios were compared to the elemental weight ratios expected for each type of material. The composition results are indicative of the known elemental weights in the target materials. The statistics are limited because of the short, 20 second data collection periods, and would improve greatly with longer exposure times in the future.

  14. Ion-Induced Afterpulsing in the Neutron Multiplicity Meter's Photomultiplier Tubes

    NASA Astrophysics Data System (ADS)

    Nedlik, Christopher; Schnee, Richard; Bunker, Raymond; Chen, Yu; Neutron Multiplicity Meter Collaboration

    2013-10-01

    The nature of the dark matter in the Universe remains a mystery in modern physics. A leading candidate, Weakly Interacting Massive Particles (WIMPs), may be detectable via scattering from nuclear targets in terrestrial detectors, located underground to prevent fake signals from cosmic-ray showers. The Neutron Multiplicity Meter (NMM) is a detector capable of measuring the muon-induced neutron flux deep underground, a problematic background for WIMP detection. The NMM is a 4.4-tonne Gd-loaded water-Cherenkov detector atop a 20-kilotonne lead target in the Soudan Mine. It measures high-energy neutrons (>50 MeV) by moderating and then detecting (via Gd capture gammas) the secondary neutrons emerging from the lead following a high-energy neutron interaction. The short time scale (~10 μs) for neutron capture in Gd-loaded water enables a custom multiplicity trigger to discriminate against the dominant gamma-ray background. Despite excellent rejection of the gamma-ray-induced background, NMM neutron-candidate events are not entirely background-free. One type of background is from ion-induced afterpulsing (AP) in the four 20'' Hamamatsu R7250 photomultiplier tubes (PMTs) used to monitor the NMM's two water tanks. We show that ion-induced AP in the PMTs can mimic the NMM's low-energy neutron response, potentially biasing a candidate event's measured multiplicity. We present detailed studies of the AP in order to allow identification of AP-induced background events.

  15. Cosmic-Ray-Induced Ship-Effect Neutron Measurements and Implications for Cargo Scanning at Borders

    SciTech Connect

    Kouzes, Richard T.; Ely, James H.; Seifert, Allen; Siciliano, Edward R.; Weier, Dennis R.; Windsor, Lindsay K.; Woodring, Mitchell L.; Borgardt, James D.; Buckley, Elise D.; Flumerfelt, Eric L.; Oliveri, Anna F.; Salvitti, Matthew

    2008-03-11

    Neutron measurements are used as part of the interdiction process for illicit nuclear materials at border crossings. Even though the natural neutron background is small, its variation can impact the sensitivity of detection systems. The natural background of neutrons that is observed in monitoring instruments arises almost entirely from cosmic ray induced cascades in the atmosphere and the surrounding environment. One significant source of variation in the observed neutron background is produced by the “ship effect” in large quantities of cargo that transit past detection instruments. This paper reports on results from measurements with typical monitoring equipment of ship effect neutrons in various materials. One new result is the “neutron shadow shielding” effect seen with some low neutron density materials.

  16. Studies of Neutron-Induced Fission of 235U, 238U, and 239Pu

    NASA Astrophysics Data System (ADS)

    Duke, Dana; TKE Team

    2014-09-01

    A Frisch-gridded ionization chamber and the double energy (2E) analysis method were used to study mass yield distributions and average total kinetic energy (TKE) release from neutron-induced fission of 235U, 238U, and 239Pu. Despite decades of fission research, little or no TKE data exist for high incident neutron energies. Additional average TKE information at incident neutron energies relevant to defense- and energy-related applications will provide a valuable observable for benchmarking simulations. The data can also be used as inputs in theoretical fission models. The Los Alamos Neutron Science Center-Weapons Neutron Research (LANSCE - WNR) provides a neutron beam from thermal to hundreds of MeV, well-suited for filling in the gaps in existing data and exploring fission behavior in the fast neutron region. The results of the studies on 238U, 235U, and 239Pu will be presented. LA-UR-14-24921.

  17. Measurement of residual 60Co activity induced by atomic-bomb neutrons in Nagasaki and background contribution by environmental neutrons.

    PubMed

    Shizuma, Kiyoshi; Endo, Satoru; Hoshi, Masaharu; Takada, Jun; Iwatani, Kazuo; Hasai, Hiromi; Oka, Takamitsu; Shimazaki, Tatsuya; Okumura, Yutaka; Fujita, Shoichiro; Watanabe, Tadaaki; Imanaka, Tetsuji

    2002-12-01

    Residual 60Co activity in five steel samples induced by neutrons from the Nagasaki atomic bomb has been measured within about 1000 m from the hypocenter. The chemical separation of cobalt and nickel from steel samples was performed, and cobalt-enriched samples were prepared for all samples. Gamma-ray measurements were carried out with a low-background well-type germanium detector. The gamma-ray spectra for five samples were compared with the spectrum of a control sample to ensure that the observed 60Co was actually induced by A-bomb neutrons. The activation of cobalt by environmental neutrons was also investigated. It has been shown that the present 60Co data are consistent with earlier Hashizume's data. PMID:12674203

  18. (n,2n) and (n,3n) cross sections of neutron-induced reactions on 150Sm for En from threshold to 35 MeV

    SciTech Connect

    Dashdorj, D; Mitchell, G; Kawano, T; Becker, J; Wu, C; Devlin, M; Fotiades, N; Nelson, R; Kunieda, S

    2009-03-16

    Cross-section measurements were made of prompt discrete {gamma}-ray production as a function of incident neutron energy (E{sub n} = 1 to 35 MeV) on a {sup 150}Sm sample fo 1550 mg/cm{sup 2} of Sm{sub 2}O{sub 3} enriched to 95.6% in {sup 150}Sm. Results are compared with enhanced Hauser-Feshbach model calculations including the pre-equilibrium reactions. Energetic neutrons were delivered by the Los Alamos Neutron Science Center facility. The prompt-reaction {gamma} rays were detected with the Compton-suppressed Germanium Array for Neutron Induced Excitations (GEANIE). Incident neutron energies were determined by the time-of-flight technique. Excitation functions for thirteen individual {gamma}-rays up to E{sub x} = 0.8 MeV in {sup 149}Sm and one {gamma}-ray transition between the first excited and ground state in {sup 148}Sm were measured. Partial {gamma}-ray cross sections were calculated using GNASH, an enhanced Hauser-Feshbach statistical nuclear reaction model code, and compared with the experimental results. The particle transmission coefficients were calculated with new systematic 'global' optical model potential parameters. The coupled-channel optical model based on the soft rotor model was employed to calculate the particle transmission coefficients. The pre-equilibrium part of the spin distribution in {sup 150}Sm was calculated using the quantum mechanical theory of Feshbach, Kerman, and Koonin (FKK) and incorporated into the GNASH reaction model code. the partial cross sections for discrete {gamma}-ray cascade paths leading to the ground state in {sup 149}Sm and {sup 148}Sm have been summed (without double counting) to estimate lower limits for reaction cross sections. These lower limits are combined with Hauser-Feshbach model calculations to deduce the reaction channel cross sections. These reaction channel cross sections agree with previously measured experimental and ENDF/B-VII evaluations.

  19. Measurement of fragment mass distributions in neutron-induced fission reactions at intermediate energies

    NASA Astrophysics Data System (ADS)

    Simutkin, V. D.; Ryzhov, I. V.; Tutin, G. A.; Vaishnene, L. A.; Blomgren, J.; Pomp, S.; Österlund, M.; Andersson, P.; Bevilacqua, R.; Meulders, J. P.; Prieels, R.

    2009-10-01

    Fragment mass distributions from neutron-induced fission of 232Th and 238U have been measured at quasi-monoenergetic neutron beam of the Louvain-la-Neuve cyclotron facility CYCLONE. The measurements have been carried out making use of a multi-section Frisch-gridded ionization chamber. The measurement technique as well as the data processing is described. Preliminary data on primary fragment mass yields are given for an incident neutron energy of 32.8 MeV.

  20. A time-gating scintillation detector for the measurement of laser-induced fast neutrons

    SciTech Connect

    Lee, Sungman; Park, Sangsoon; Yea, Kwon-hae; Cha, Hyungki

    2009-06-15

    A time-gating scintillation detector, in which a fast high voltage switch is used for gating a channel photomultiplier, was developed for a measurement of laser-induced fast neutrons. The x rays generated from the intense femtosecond laser and the solid target interactions were suppressed selectively and a time-of-flight signal of a laser-generated fast neutron was measured effectively. The detector was used successfully to measure the neutron yield of a femtosecond, deuterated, polystyrene plasma.

  1. A time-gating scintillation detector for the measurement of laser-induced fast neutrons.

    PubMed

    Lee, Sungman; Park, Sangsoon; Yea, Kwon-hae; Cha, Hyungki

    2009-06-01

    A time-gating scintillation detector, in which a fast high voltage switch is used for gating a channel photomultiplier, was developed for a measurement of laser-induced fast neutrons. The x rays generated from the intense femtosecond laser and the solid target interactions were suppressed selectively and a time-of-flight signal of a laser-generated fast neutron was measured effectively. The detector was used successfully to measure the neutron yield of a femtosecond, deuterated, polystyrene plasma. PMID:19566199

  2. Energy- and time-resolved detection of prompt gamma-rays for proton range verification

    NASA Astrophysics Data System (ADS)

    Verburg, Joost M.; Riley, Kent; Bortfeld, Thomas; Seco, Joao

    2013-10-01

    In this work, we present experimental results of a novel prompt gamma-ray detector for proton beam range verification. The detection system features an actively shielded cerium-doped lanthanum(III) bromide scintillator, coupled to a digital data acquisition system. The acquisition was synchronized to the cyclotron radio frequency to separate the prompt gamma-ray signals from the later-arriving neutron-induced background. We designed the detector to provide a high energy resolution and an effective reduction of background events, enabling discrete proton-induced prompt gamma lines to be resolved. Measuring discrete prompt gamma lines has several benefits for range verification. As the discrete energies correspond to specific nuclear transitions, the magnitudes of the different gamma lines have unique correlations with the proton energy and can be directly related to nuclear reaction cross sections. The quantification of discrete gamma lines also enables elemental analysis of tissue in the beam path, providing a better prediction of prompt gamma-ray yields. We present the results of experiments in which a water phantom was irradiated with proton pencil-beams in a clinical proton therapy gantry. A slit collimator was used to collimate the prompt gamma-rays, and measurements were performed at 27 positions along the path of proton beams with ranges of 9, 16 and 23 g cm-2 in water. The magnitudes of discrete gamma lines at 4.44, 5.2 and 6.13 MeV were quantified. The prompt gamma lines were found to be clearly resolved in dimensions of energy and time, and had a reproducible correlation with the proton depth-dose curve. We conclude that the measurement of discrete prompt gamma-rays for in vivo range verification of clinical proton beams is feasible, and plan to further study methods and detector designs for clinical use.

  3. Neutron-induced fission cross sections of short-lived actinides with the surrogate reaction method.

    SciTech Connect

    Kessedijian, G.; Jurado, B.; Aiche, M.; Barreau, G.; Bidaud, A.; Czajkowski, S.; Dassie, D.; Haas, B.; Mathieu, L.; Audouin, L.; Capellan, N.; Tassan-Got, L.; Wilson, J. N.; Berthoumieux, E.; Gunsing, F.; Theisen, Ch.; Serot, O.; Bauge, E.; Ahmad, I.; Greene, J. P.; Janssens, R. V. F.

    2010-09-13

    Neutron-induced fission cross sections for {sup 242,243}Cm and {sup 241}Am have been obtained with the surrogate reaction method. Recent results for the neutron-induced cross section of {sup 243}Cm are questioned by the present data. For the first time, the {sup 242}Cm cross section has been determined up to the onset of second-chance fission. The good agreement at the lowest excitation energies between the present results and the existing neutron-induced data indicates that the distributions in spin and parity of states populated with both techniques are similar.

  4. Effects of hole doping by neutron irradiation of magnetic field induced electronic phase transitions in graphite

    SciTech Connect

    Singleton, John; Yaguchi, Hiroshi

    2008-01-01

    We have investigated effects of hole doping by fast-neutron irradiation on the magnetic-field induced phase transitions in graphite using specimens irradiated with fast neutrons. Resistance measurements have been done in magnetic fields of up to above 50 T and at temperatures down to about 1.5 K. The neutron irradiation creates lattice defects acting as acceptors, affecting the imbalance of the electron and hole densities and the Fermi level. We have found that the reentrant field from the field induced state back to the normal state shifts towards a lower field with hole doping, suggestive of the participation of electron subbands in the magnetic-field induced state.

  5. Study of muon-induced neutron production using accelerator muon beam at CERN

    SciTech Connect

    Nakajima, Y.; Lin, C. J.; Ochoa-Ricoux, J. P.; Draeger, E.; White, C. G.; Luk, K. B.; Steiner, H.

    2015-08-17

    Cosmogenic muon-induced neutrons are one of the most problematic backgrounds for various underground experiments for rare event searches. In order to accurately understand such backgrounds, experimental data with high-statistics and well-controlled systematics is essential. We performed a test experiment to measure muon-induced neutron production yield and energy spectrum using a high-energy accelerator muon beam at CERN. We successfully observed neutrons from 160 GeV/c muon interaction on lead, and measured kinetic energy distributions for various production angles. Works towards evaluation of absolute neutron production yield is underway. This work also demonstrates that the setup is feasible for a future large-scale experiment for more comprehensive study of muon-induced neutron production.

  6. The Status of Cross Section Measurements for Neutron-induced Reactions Needed for Cosmic Ray Studies

    NASA Technical Reports Server (NTRS)

    Sisterson, J. M.

    2003-01-01

    Cosmic ray interactions with lunar rocks and meteorites produce small amounts of radionuclides and stable isotopes. Advances in Accelerator Mass Spectrometry (AMS) allow production rates to be measured routinely in well-documented lunar rocks and meteorites. These measurements are analyzed using theoretical models to learn about the object itself and the history of the cosmic rays that fell on it. Good cross section measurements are essential input to the theoretical calculations. Most primary cosmic ray particles are protons so reliable cross sections for proton-induced reactions are essential. A cross section is deemed accurate if measurements made by different experimenters using different techniques result in consistent values. Most cross sections for proton induced reactions are now well measured. However, good cross section measurements for neutron-induced reactions are still needed. These cross sections are required to fully account for all galactic cosmic ray interactions at depth in an extraterrestrial object. When primary galactic cosmic ray (GCR) particles interact with an object many secondary neutrons are produced, which also initiate spallation reactions. Thus, the total GCR contribution to the overall cosmogenic nuclide archive has to include the contribution from the secondary neutron interactions. Few relevant cross section measurements have been reported for neutron-induced reactions at neutron energies greater than approximately 20 MeV. The status of the cross section measurements using quasi-monoenergetic neutron energies at iThemba LABS, South Africa and white neutron beams at Los Alamos Neutron Science Center (LANSCE), Los Alamos are reported here.

  7. Radioactive targets for neutron-induced cross section measurements

    SciTech Connect

    Kronenberg, A.; Bond, E. M.; Glover, S. E.; Rundberg, R. S.; Vieira, D. J.; Esch, E. I.; Reifarth, R.; Ullmann, J. L.; Haight, Robert C.; Rochmann, D.

    2004-01-01

    Measurements using radioactive targets are important for the determination of key reaction path ways associated with the synthesis of the elements in nuclear astrophysics (sprocess), advanced fuel cycle initiative (transmutation of radioactive waste), and stockpile stewardship. High precision capture cross-section measurements are needed to interpret observations, predict elemental or isotopical ratios, and unobserved abundances. There are two new detector systems that are presently being commissioned at Los Alamos National Laboratory for very precise measurements of (n,{gamma}) and (n,f) cross-sections using small quantities of radioactive samples. DANCE (Detector for Advanced Neutron-Capture Experiments), a 4 {pi} gamma array made up of 160 BaF{sub 2} detectors, is designed to measure neutron capture cross-sections of unstable nuclei in the low-energy range (thermal to {approx}500 keV). The high granularity and high detection efficiency of DANCE, combined with the high TOF-neutron flux available at the Lujan Center provides a versatile tool for measuring many important cross section data using radioactive and isotopically enriched targets of about 1 milligram. Another powerful instrument is the Lead-slowing down spectrometer (LSDS), which will enable the measurement of neutron-induced fission cross-section of U-235m and other short-lived actinides in a energy range from 1-200 keV with sample sizes down to 10 nanograms. Due to the short half-life of the U-235m isomer (T{sub 1/2} = 26 minutes), the samples must be rapidly and repeatedly extracted from its {sup 239}Pu parent. Since {sup 239}Pu is itself highly fissile, the separation must not only be rapid, but must also be of very high purity (the Pu must be removed from the U with a decontamination factor >10{sup 12}). Once extracted and purified, the {sup 235m}U isomer would be electrodeposited on solar cells as a fission detector and placed within the LSDS for direct (n,f) cross section measurements. The

  8. Neutron-induced soft error rate measurements in semiconductor memories

    NASA Astrophysics Data System (ADS)

    Ünlü, Kenan; Narayanan, Vijaykrishnan; Çetiner, Sacit M.; Degalahal, Vijay; Irwin, Mary J.

    2007-08-01

    Soft error rate (SER) testing of devices have been performed using the neutron beam at the Radiation Science and Engineering Center at Penn State University. The soft error susceptibility for different memory chips working at different technology nodes and operating voltages is determined. The effect of 10B on SER as an in situ excess charge source is observed. The effect of higher-energy neutrons on circuit operation will be published later. Penn State Breazeale Nuclear Reactor was used as the neutron source in the experiments. The high neutron flux allows for accelerated testing of the SER phenomenon. The experiments and analyses have been performed only on soft errors due to thermal neutrons. Various memory chips manufactured by different vendors were tested at various supply voltages and reactor power levels. The effect of 10B reaction caused by thermal neutron absorption on SER is discussed.

  9. Calculations of neutron flux spectra induced in the earth's atmosphere by galactic cosmic rays

    NASA Technical Reports Server (NTRS)

    Armstrong, T. W.; Chandler, K. C.; Barish, J.

    1972-01-01

    Calculations have been carried out to determine the neutron flux induced in the earth's atmosphere by galactic protons and alpha particles at solar minimum for a geomagnetic latitude of 42 N. Neutron flux spectra were calculated using Monte Carlo and discrete ordinates methods, and various comparisons with experimental data are presented. The magnitude and shape of the calculated neutron-leakage spectrum at the particular latitude considered support the theory that the cosmic-ray-albedo-neutron-decay mechanism is the source of the protons and electrons trapped in the Van Allen belts.

  10. Neutron-induced 2.2 MeV background in gamma ray telescopes

    NASA Technical Reports Server (NTRS)

    Zanrosso, E. M.; Long, J. L.; Zych, A. D.; White, R. S.

    1985-01-01

    Neutron-induced gamma ray production is an important source of background in Compton scatter gamma ray telescopes where organic scintillator material is used. Most important is deuteron formation when atmospheric albedo and locally produced neutrons are thermalized and subsequently absorbed in the hydrogenous material. The resulting 2.2 MeV gamma ray line radiation essentially represents a continuous isotropic source within the scintillator itself. Interestingly, using a scintillator material with a high hydrogen-to-carbon ratio to minimize the scintillator material with a high hydrogen-to-carbon ratio to minimize the neutron-induced 4.4 MeV carbon line favors the np reaction. The full problem of neutron-induced background in Compton scatter telescopes has been previously discussed. Results are presented of observations with the University of California balloon-borne Compton scatter telescope where the 2.2 MeV induced line emission is prominently seen.

  11. Radioactivity induced by neutrons: Enrico Fermi and a thermodynamic approach to radiative capture

    NASA Astrophysics Data System (ADS)

    De Gregorio, Alberto

    2006-07-01

    When Fermi learned that slow neutrons are much more effective than fast ones in inducing radioactivity, he explained this phenomenon by mentioning the well-known scattering cross section between neutrons and protons. At this early stage, he did not refer to the capture cross section by target nuclei. At the same time a thermodynamic approach to neutron-proton capture was being discussed by physicists: neutron capture was interpretated as the reverse of deuteron photodissociation and detailed balance among neutrons, protons, deuterons, and radiation was invoked. This thermodynamic approach might underlie Fermi's early explanation of the great efficiency of slow neutrons. Fermi repeatedly used a thermodynamic approach that had been used in describing some of the physical properties of conductors by Richardson and had been influential in Fermi's youth.

  12. Neutron Induced Capture Reaction Studies in the Resonance Region at GELINA

    SciTech Connect

    Schillebeeckx, Peter; Borella, A.; Kopecky, S.; Mihailescu, L. C.; Siegler, P.; Sirakov, I.; Massimi, C.; Moxon, M.; Ware, T.

    2009-01-28

    The neutron time-of-flight facility GELINA installed at the IRMM Geel (B) has been designed to study neutron-induced reactions in the resonance region. It is a multi-user facility, providing a pulsed white neutron source, with a neutron energy range between 10 meV and 20 MeV and a time resolution of 1 ns. The research program concentrates on cross section data needs for nuclear energy applications. In this paper efforts to improve the quality of cross section data for neutron induced capture reactions in the resolved and unresolved resonance region are presented together with examples of cross section data to support the development of advanced reactor concepts and to optimize the use of present nuclear power plants.

  13. Modeling of Time-correlated Detection of Fast Neutrons Emitted in Induced SNM Fission

    NASA Astrophysics Data System (ADS)

    Guckes, Amber; Barzilov, Alexander; Richardson, Norman

    Neutron multiplicity methods are widely used in the assay of fissile materials. Fission reactions release multiple neutrons simultaneously. Time-correlated detection of neutrons provides a coincidence signature that is unique to fission,which enables distinguishing it from other events. In general, fission neutrons are fast. Thermal neutron sensors require the moderation of neutrons prior to a detection event; therefore, the neutron's energy and the event's timing information may be distorted, resulting in the wide time windows in the correlation analysis. Fastneutron sensing using scintillators allows shortening the time correlation window. In this study, four EJ-299-33A plastic scintillator detectors with neutron/photon pulse shape discrimination properties were modeled usingthe MCNP6 code. This sensor array was studied for time-correlated detection of fast neutrons emitted inthe induced fission of 239Pu and (α,n) neutron sources. This paper presents the results of computational modeling of arrays of these plastic scintillator sensors as well as3He detectors equipped with a moderator.

  14. Comparing the Effects of Echoic Prompts and Echoic Prompts Plus Modeled Prompts on Intraverbal Behavior

    ERIC Educational Resources Information Center

    Valentino, Amber L.; Shillingsburg, M. Alice; Call, Nathan A.

    2012-01-01

    We compared strategies to teach vocal intraverbal responses to an adolescent diagnosed with autism and Down syndrome. One strategy involved echoic prompts only. The second strategy involved an echoic prompt paired with a modeled prompt in the form of sign language. Presenting the modeled prompt with the echoic prompt resulted in faster acquisition…

  15. Neutron induced soft errors in CMOS memories under reduced bias

    SciTech Connect

    Hazucha, P.; Svensson, C.; Johansson, K.

    1998-12-01

    A custom designed 16 kbit CMOS memory was irradiated by 14 MeV neutrons and 100 MeV neutrons. SEU cross sections were evaluated under different supply voltages. The cross section values are compared to those predicted by the BGR model.

  16. Dynamical simulation of neutron-induced fission of uranium isotopes using four-dimensional Langevin equations

    NASA Astrophysics Data System (ADS)

    Pahlavani, M. R.; Mirfathi, S. M.

    2016-04-01

    Four-dimensional Langevin equations have been suggested for the dynamical simulation of neutron-induced fission at low and medium excitation energies. The mass distribution of the fission fragments, the neutron multiplicity, and the fission cross section for the thermal and fast neutron-induced fission of 233U, 235U, and 238U is studied by considering energy dissipation of the compound nucleus through the fission using four-dimensional Langevin equations combined with a Monte Carlo simulation approach. The calculated results using this approach indicate reasonable agreement with available experimental data.

  17. Flux and dose transmission through concrete of neutrons from proton induced reactions on various target elements

    NASA Astrophysics Data System (ADS)

    Maiti, Moumita; Nandy, Maitreyee; Roy, S. N.; Sarkar, P. K.

    2004-12-01

    Simple empirical expressions for transmission of flux and dose through concrete are presented for neutrons from proton induced reactions. For this purpose the neutron emission from different targets in proton induced reactions in the energy range 25-200 MeV have been considered. The calculated effective dose outside a concrete shield shows overall good agreement with the effective dose estimated from measured neutron flux in the framework of the Moyer model. The calculated effective attenuation length shows a rising trend with incident proton energy and shield thickness.

  18. Laser induced neutron production by explosion of the deuterium clusters

    NASA Astrophysics Data System (ADS)

    Holkundkar, Amol R.; Mishra, Gaurav; Gupta, N. K.

    2014-01-01

    The high energy deuterium ions serve as compact source of neutrons when fused with either deuterium or tritium atoms. In view of this, the explosion of the deuterium clusters under the influence of the laser pulse with intensity ranging from 1015 to 1019 W/cm2 is being studied along with the effect of the cluster radius and inter-cluster distance. The objective of this article is to study the efficiency of the deuterium cluster as a compact source of neutrons under various laser and cluster parameters. It is being observed that the cluster density (number of clusters per unit volume) is quite important to gain high neutron yield.

  19. Fusion probability for neutron-rich radioactive Sn induced reactions

    SciTech Connect

    Liang, J Felix; Gross, Carl J; Kohley, Zachary W; Shapira, Dan; Varner Jr, Robert L; Allmond, James M; Caraley, Anne L; Lagergren, Karin B; Mueller, Paul Edward

    2012-01-01

    Evaporation residue cross sections for $^{124,126,127,128}$Sn+$^{64}$Ni and $^{132}$Sn+$^{58}$Ni have been measured to study the effects of neutron excess in neutron-rich radioactive nuclei on fusion. For the reactions with $^{64}$Ni, the fusion probability does not decrease with increasing neutron excess in Sn, contrary to the result of the stable beam Sn+Zr measurement. A comparison of the reduced evaporation residue cross sections for $^{126}$Sn+$^{64}$Ni and $^{132}$Sn+$^{58}$Ni, which make the same compound nucleus, shows that the fusion probability is indistinguishable for reactions involving the same atomic elements but different isotope combinations.

  20. Neutron induced background in the COMPTEL detector on the Gamma Ray Observatory

    NASA Technical Reports Server (NTRS)

    Morris, D. J.; Aarts, H.; Bennett, K.; Busetta, M.; Byrd, R.; Collmar, W.; Connors, A.; Diehl, R.; Eymann, G.; Foster, C.

    1992-01-01

    Interactions of neutrons in a prototype of the Compton imaging telescope (COMPTEL) gamma ray detector for the Gamma Ray Observatory were studied to determine COMPTEL's sensitivity as a neutron telescope and to estimate the gamma ray background resulting from neutron interactions. The IUCF provided a pulsed neutron beam at five different energies between 18 and 120 MeV. These measurements showed that the gamma ray background from neutron interactions is greater than previously expected. It was thought that most such events would be due to interactions in the upper detector modules of COMPTEL and could be distinguished by pulse shape discrimination. Rather, the bulk of the gamma ray background appears to be due to interactions in passive material, primarily aluminum, surrounding the D1 modules. In a considerable fraction of these interactions, two or more gamma rays are produced simultaneously, with one interacting in the D1 module and the other interacting in the module of the lower (D2) detector. If the neutron interacts near the D1 module, the D1 D2 time of flight cannot distinguish such an event from a true gamma ray event. In order to assess the significance of this background, the flux of neutrons in orbit has been estimated based on observed events with neutron pulse shape signature in D1. The strength of this neutron induced background is estimated. This is compared with the rate expected from the isotropic cosmic gamma ray flux.

  1. A laser-induced repetitive fast neutron source applied for gold activation analysis

    NASA Astrophysics Data System (ADS)

    Lee, Sungman; Park, Sangsoon; Lee, Kitae; Cha, Hyungki

    2012-12-01

    A laser-induced repetitively operated fast neutron source was developed for applications in laser-driven nuclear physics research. The developed neutron source, which has a neutron yield of approximately 4 × 105 n/pulse and can be operated up to a pulse repetition rate of 10 Hz, was applied for a gold activation analysis. Relatively strong delayed gamma spectra of the activated gold were measured at 333 keV and 355 keV, and proved the possibility of the neutron source for activation analyses. In addition, the nuclear reactions responsible for the measured gamma spectra of gold were elucidated by the 14 MeV fast neutrons resulting from the D(t,n)He4 nuclear reaction, for which the required tritium originated from the primary fusion reaction, D(d,p)T3.

  2. A laser-induced repetitive fast neutron source applied for gold activation analysis

    SciTech Connect

    Lee, Sungman; Park, Sangsoon; Lee, Kitae; Cha, Hyungki

    2012-12-15

    A laser-induced repetitively operated fast neutron source was developed for applications in laser-driven nuclear physics research. The developed neutron source, which has a neutron yield of approximately 4 Multiplication-Sign 10{sup 5} n/pulse and can be operated up to a pulse repetition rate of 10 Hz, was applied for a gold activation analysis. Relatively strong delayed gamma spectra of the activated gold were measured at 333 keV and 355 keV, and proved the possibility of the neutron source for activation analyses. In addition, the nuclear reactions responsible for the measured gamma spectra of gold were elucidated by the 14 MeV fast neutrons resulting from the D(t,n)He{sup 4} nuclear reaction, for which the required tritium originated from the primary fusion reaction, D(d,p)T{sup 3}.

  3. A laser-induced repetitive fast neutron source applied for gold activation analysis.

    PubMed

    Lee, Sungman; Park, Sangsoon; Lee, Kitae; Cha, Hyungki

    2012-12-01

    A laser-induced repetitively operated fast neutron source was developed for applications in laser-driven nuclear physics research. The developed neutron source, which has a neutron yield of approximately 4 × 10(5) n/pulse and can be operated up to a pulse repetition rate of 10 Hz, was applied for a gold activation analysis. Relatively strong delayed gamma spectra of the activated gold were measured at 333 keV and 355 keV, and proved the possibility of the neutron source for activation analyses. In addition, the nuclear reactions responsible for the measured gamma spectra of gold were elucidated by the 14 MeV fast neutrons resulting from the D(t,n)He(4) nuclear reaction, for which the required tritium originated from the primary fusion reaction, D(d,p)T(3). PMID:23277984

  4. Neutron-fragment and Neutron-neutron Correlations in Low-energy Fission

    NASA Astrophysics Data System (ADS)

    Lestone, J. P.

    2016-01-01

    A computational method has been developed to simulate neutron emission from thermal-neutron induced fission of 235U and from spontaneous fission of 252Cf. Measured pre-emission mass-yield curves, average total kinetic energies and their variances, both as functions of mass split, are used to obtain a representation of the distribution of fragment velocities. Measured average neutron multiplicities as a function of mass split and their dependence on total kinetic energy are used. Simulations can be made to reproduce measured factorial moments of neutron-multiplicity distributions with only minor empirical adjustments to some experimental inputs. The neutron-emission spectra in the rest-frame of the fragments are highly constrained by ENDF/B-VII.1 prompt-fission neutron-spectra evaluations. The n-f correlation measurements of Vorobyev et al. (2010) are consistent with predictions where all neutrons are assumed to be evaporated isotropically from the rest frame of fully accelerated fragments. Measured n-f and n-n correlations of others are a little weaker than the predictions presented here. These weaker correlations could be used to infer a weak scission-neutron source. However, the effect of neutron scattering on the experimental results must be studied in detail before moving away from a null hypothesis that all neutrons are evaporated from the fragments.

  5. Neutron-Induced Fission Measurements at the Dance and Lsds Facilities at Lanl

    NASA Astrophysics Data System (ADS)

    Jandel, M.; Bredeweg, T. A.; Bond, E. M.; Chadwick, M. B.; Couture, A.; O'Donnell, J. M.; Fowler, M. M.; Haight, R. C.; Hayes-Sterbenz, A. C.; Rundberg, R. S.; Rusev, G. Y.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wu, C. Y.; Becker, J. A.; Alexander, C. W.; Belier, G.

    2014-09-01

    New results from neutron-induced fission measurements performed at the Detector for Advanced Neutron Capture Experiments (DANCE) and Lead Slowing Down Spectrometer (LSDS) are presented. New correlated data on promptfission γ-ray (PFG) distributions were measured using the DANCE array for resonant neutron-induced fission of 233U, 235U and 239Pu. The deduced properties of PFG emission are presented using a simple parametrization. An accurate knowledge of fission γ-ray spectra enables us to analyze the isomeric states of 236U created after neutron capture on 235U. We briefly discuss these new results. Finally, we review details and preliminary results of the challenging 237U(n,f) cross section measurement at the LSDS facility.

  6. Neutron induced pion production on C, Al, Cu, and W at neutron energies of 200--600 MeV

    SciTech Connect

    Brooks, M.L.

    1991-10-01

    Inclusive double differential neutron induced {pi}{sup +} and {pi}{sup {minus}} production cross sections were measured for four separate targets: C, Al, Cu and W. The neutron energy range was 200--600 MeV and the pion angular range was 25{degrees}--125{degrees}. The charge, scattering angle and energy of the pions were measured using a magnetic spectrometer. The measurements are compared with intranuclear cascade (INC) calculations and a previous experiment that measured the sum of the {pi}{sup +} and {pi}{sup {minus}} cross sections. Our data agree with the measured data, but the INC calculations give only moderate agreement with the double differential cross sections as well as with angular distributions and total cross sections as a function of neutron energy. The ratio of {pi}{sup {minus}}:{pi}{sup +} was found to increase rapidly with decreasing neutron energy and the pion production was found to increase approximately as A{sup 2/3} for the different targets. 31 refs., 55 figs., 6 tabs.

  7. AttoPhotoChemistry. Probing ultrafast electron dynamics by the induced nuclear motion: The prompt and delayed predissociation of N2

    NASA Astrophysics Data System (ADS)

    Muskatel, B. H.; Remacle, F.; Levine, R. D.

    2014-05-01

    Quantum mechanical wavepacket dynamics simulation that includes the nuclear motion exhibit a prompt, few fs, dissociation of electronically attosecond excited N2 in addition to the slow dissociation evident from spectral line broadening in well resolved spectra. The simulations show that nuclear motion can probe early times electron dynamics. The separation of time scales is mimicked by a model study fashioned like chemical kinetics of unimolecular dissociation. The physical origin of the separation into prompt and delayed decay is argued to be the same in the vibrational and the present case, namely that there are more bound than dissociative channels.

  8. Activation analysis of indium, KCl, and melamine by using a laser-induced neutron source

    NASA Astrophysics Data System (ADS)

    Lee, Sungman; Lee, Kitae; Cha, Hyungki

    2014-04-01

    A laser-induced repetitively operated fast neutron source with a neutron yield of 4 × 105 n/pulse and a pulse repetition rate of 5 Hz, which was developed using a deuterated polystyrene film target and a 24-TW femtosecond laser, was applied for laser activation analyses of indium, KCl, and melamine samples. The nuclear reactions of the measured gamma spectra for the activated samples were identified as (n, γ), (n, n'), and (n, 2n) reactions. These indicate possible usage of the neutron source for practical activation analyses of various materials.

  9. Experimental study of neutron induced background noise on gated x-ray framing cameras

    SciTech Connect

    Izumi, N.; Hagmann, C.; Stone, G.; Hey, D.; Glenn, S.; Conder, A.; Teruya, A.; Sorce, C.; Tommasini, R.; Stoeffl, W.; Springer, P.; Landen, O. L.; Eckart, M.; Mackinnon, A. J.; Koch, J. A.; Bradley, D. K.; Bell, P.; Herrmann, H. W.; Kyrala, G. A.; Bahukutumbi, R.; and others

    2010-10-15

    A temporally gated x-ray framing camera based on a proximity focus microchannel plate is one of the most important diagnostic tools of inertial confinement fusion experiments. However, fusion neutrons produced in imploded capsules interact with structures surrounding the camera and produce background to x-ray signals. To understand the mechanisms of this neutron induced background, we tested several gated x-ray cameras in the presence of 14 MeV neutrons produced at the Omega laser facility. Differences between background levels observed with photographic film readout and charge-coupled-device readout have been studied.

  10. Loud and Bright: Gravitational and possible electromagnetic signals induced by binary neutron star mergers

    NASA Astrophysics Data System (ADS)

    Palenzuela, Carlos; Lehner, Luis; Ponce, Marcelo; Thompson, Chris; Liebling, Steve; Neilsen, Dave; Hirschmann, Eric; Anderson, Matt; Motl, Patrick

    2013-04-01

    Our main goal is to investigate how the strongly gravitating and highly dynamical behavior of magnetized binary neutron stars can affect the plasma in the magnetosphere in such a way that powerful electromagnetic emissions can be induced, as well as stressing its connection with gravitational waves produced by the system. Such phenomena is a natural candidate for bright (EM) and loud (GW) emissions, as pulsars are strong electromagnetic emitters on one hand, and merging binary neutron stars are powerful sources of gravitational radiation.

  11. Neutron-induced fission measurements at the time-of-flight facility nELBE

    DOE PAGESBeta

    Kögler, T.; Beyer, R.; Junghans, A. R.; Massarczyk, R.; Schwengner, R.; Wagner, A.

    2015-05-18

    Neutron-induced fission of ²⁴²Pu is studied at the photoneutron source nELBE. The relative fast neutron fission cross section was determined using actinide fission chambers in a time-of-flight experiment. A good agreement of present nuclear data with evalua- tions has been achieved in the range of 100 keV to 10 MeV.

  12. Studies of near-barrier fusion induced by neutron-rich nuclei at HRIBF

    SciTech Connect

    Liang, J Felix

    2011-01-01

    Fusion induced by neutron-rich radioactive beams is a topic of current interest. The findings will be useful for using radioactive beams to produce superheavy elements. Results from recent measurements performed with neutron-rich radioactive Sn and Te beams are presented. Coupled-channels calculations were carried out to study the observed sub-barrier fusion enhancement. The fusion probability in Sn on Ni were probed by comparing the evaporation residue cross sections at high excitation energies.

  13. Laser induced neutron production by explosion of the deuterium clusters

    SciTech Connect

    Holkundkar, Amol R.; Mishra, Gaurav Gupta, N. K.

    2014-01-15

    The high energy deuterium ions serve as compact source of neutrons when fused with either deuterium or tritium atoms. In view of this, the explosion of the deuterium clusters under the influence of the laser pulse with intensity ranging from 10{sup 15} to 10{sup 19} W/cm{sup 2} is being studied along with the effect of the cluster radius and inter-cluster distance. The objective of this article is to study the efficiency of the deuterium cluster as a compact source of neutrons under various laser and cluster parameters. It is being observed that the cluster density (number of clusters per unit volume) is quite important to gain high neutron yield.

  14. Reactions induced by beams of neutron and proton halo nuclei

    NASA Astrophysics Data System (ADS)

    Penionzhkevich, Yu. E.

    1997-02-01

    Within the collaboration Dubna-GANIL (Caen, France) - IPN (Orsay, France) - NPI (Rez, Czech Republic) - IAP (Bucharest, Romania) at GANIL and the Dubna U400M accelerator, experiments have been carried out to study elastic scattering, fusion and fission using secondary ion beams of 6He, 11Li and 8B. The fission cross-section for the 6He isotopes has been found to be significantly higher than for the 4He nuclei. This enhancement depends mainly on the entrance channel and it is connected with the neutron skin of the 6He nuclei. Also, investigation of the elastic scattering of 11Li (neutron halo), 7Be and 8B (proton halo) has been performed. The microscopic analysis supports the existence of a neutron halo in 11Li and the proton skin in 8B and 7Be. Perspectives for investigations in this field at the Laboratory of Nuclear Reactions JINR are also discussed.

  15. New Measurements of Fission Neutron Spectra at Intermediate Energies

    NASA Astrophysics Data System (ADS)

    Ethvignot, Thierry; Granier, Thierry; Haight, Robert C.; O'Donnell, John M.; Devlin, Matthew; Nelson, Ronald O.; Drosg, Roswitha

    2002-04-01

    Interest in obtaining a more detailed understanding of prompt neutron emission in fission is now high. Information on neutron-induced fission of actinides for incident-neutron energies from a few MeV to higher energies, except for data at 14 MeV is sparse. Such measurements are now possible, and the data are needed for design studies of accelerator-driven systems. Moreover, these data provide valuable information to improve our understanding of fission at high excitation energy. As a matter of fact, a theoretical effort has been pursued recently to predict the properties of prompt neutron emission in fission. They are characterized by two basic quantities, the average number of prompt neutrons emitted per fission, which is well known up to 20 MeV, and the neutron energy spectrum, which is not nearly so well known. However, it was shown for a few cases that not only the average energy but also the shape of the Fission Neutron Spectra (FNS) depend on the incident neutron energy. It is particularly interesting to investigate the change in shape of the FNS around the first, second and third chance fission where the properties of the fissioning nucleus drastically change. At the WNR white source, the FNS were measured with the FIGARO set-up, with a ^238U fission chamber as the target. Both incoming and emitted neutron energies were determined with their time of flight. Preliminary results of recorded spectra will be presented at the meeting.

  16. Optomechanical design of a prompt gamma reaction history diagnostic

    SciTech Connect

    Hermann, Hans W; Kaufman, Morris I; Malone, Robert M; Frogget, Brent C; Tunnell, Thomas W; Cox, Brian; Frayer, Daniel K; Ali, Zaheer; Stoeffl, Wolfgang

    2009-01-01

    The National Ignition Facility and the Omega Laser Facility both have a need for measuring prompt gamma radiation as part of a nuclear diagnostic program. A new gamma-detection diagnostic using off-axis-parabolic mirrors has been built. Some new techniques were used in the design, construction, and tolerancing of this gamma ray diagnostic. Because of the wavelength requirement (250-700 nm), the optical element surface finishes were a key design consideration. The optical enclosure had to satisfy pressure safety concerns and shielding against electromagnetic interference induced by gammas and neutrons. Structural finite element analysis was needed to meet rigorous optical and safety requirements. The optomechanical design is presented. Alignment issues are also discussed.

  17. Neutron induced radio-isotopes and background for Ge double beta decay experiments

    NASA Astrophysics Data System (ADS)

    Chu, Pinghan; Majorana Collaboration

    2015-10-01

    Environmental neutrons, mostly produced by muons in the cosmic rays, might contribute backgrounds to the search for neutrinoless double beta decays. These neutrons can interact with materials and generate radio-isotopes, which can decay and produce radioactive backgrounds. Some of these neutron-induced isotopes have a signature of a time-delayed coincidence, allowing us to study these infrequent events. For example, such isotopes can decay by beta decay to metastable states and then decay by gamma decay to the ground state. Considering the time-delayed coincidence of these two processes, we can determine candidates for these neutron-induced isotopes in the data and estimate the flux of neutrons in the deep underground environment. In this report, we will list possible neutron-induced isotopes and the methodology to detect them, especially those that can affect the search for neutrinoless double beta decays in 76Ge. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, the Particle Astrophysics Program of the National Science Foundation, and the Sanford Underground Research Facility. We acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program.

  18. Neutrons scattering studies in the actinide region

    SciTech Connect

    Kegel, G.H.R.; Egan, J.J.

    1992-09-01

    During the report period were investigated the following areas: prompt fission neutron energy spectra measurements; neutron elastic and inelastic scattering from [sup 239]Pu; neutron scattering in [sup 181]Ta and [sup 197]Au; response of a [sup 235]U fission chamber near reaction thresholds; two-parameter data acquisition system; black'' neutron detector; investigation of neutron-induced defects in silicon dioxide; and multiple scattering corrections. Four Ph.D. dissertations and one M.S. thesis were completed during the report period. Publications consisted of three journal articles, four conference papers in proceedings, and eleven abstracts of presentations at scientific meetings. There are currently four Ph.D. and one M.S. candidates working on dissertations directly associated with the project. In addition, three other Ph.D. candidates are working on dissertations involving other aspects of neutron physics in this laboratory.

  19. Neutrons scattering studies in the actinide region

    NASA Astrophysics Data System (ADS)

    Kegel, G. H. R.; Egan, J. J.

    1992-09-01

    During the last report period, we investigated the following areas: prompt fission neutron energy spectra measurements; neutron elastic and inelastic scattering from Pu-239; neutron scattering in Ta-181 and Au-197; response of a U-235 fission chamber near reaction thresholds; two-parameter data acquisition system; 'black' neutron detector; investigation of neutron-induced defects in silicon dioxide; and multiple scattering corrections. Four Ph.D. dissertations and one M.S. thesis were completed during the report period. Publications consisted of three journal articles, four conference papers in proceedings, and eleven abstracts of presentations at scientific meetings. There are currently four Ph.D. and one M.S. candidates working on dissertations directly associated with the project. In addition, three other Ph.D. candidates are working on dissertations involving other aspects of neutron physics in this laboratory.

  20. Neutron-induced reactions in tissue-resident elements

    SciTech Connect

    Herling, G.H.; Bassel, R.H.; Adams, J.H.; Fraser, W.A.

    1981-07-08

    Kerma-to-fluence ratios have been calculated for neutrons with energies between 20 and 60 MeV incident upon 1H, 12C, 14N, and 16O. The following charged particles have been taken into account: protons, deuterons, alpha particles, and heavy recoils. Results are presented for NE-213 plastic, muscle, and tissue-equivalent plastic.

  1. Neutron-induced reactions in the hohlraum to study reaction in flight neutrons

    NASA Astrophysics Data System (ADS)

    Boswell, M. S.; Elliott, S. R.; Guiseppe, V.; Kidd, M.; Rundberg, B.; Tybo, J.

    2013-04-01

    We are currently developing the physics necessary to measure the Reaction In Flight (RIF) neutron flux from a NIF capsule. A measurement of the RIF neutron flux from a NIF capsule could be used to deduce the stopping power in the cold fuel of the NIF capsule. A foil irradiated at the Omega laser at LLE was counted at the LANL low-background counting facility at WIPP. The estimated production rate of 195Au was just below our experimental sensitivity. We have made several improvements to our counting facility in recent months. These improvements are designed to increase our sensitivity, and include installing two new low-background detectors, and taking steps to reduce noise in the signals.

  2. Neutron-induced reactions in the hohlraum to study reaction in flight neutrons

    SciTech Connect

    Boswell, M. S.; Elliott, S. R.; Tybo, J.; Guiseppe, V.; Rundberg, B.; Kidd, M.

    2013-04-19

    We are currently developing the physics necessary to measure the Reaction In Flight (RIF) neutron flux from a NIF capsule. A measurement of the RIF neutron flux from a NIF capsule could be used to deduce the stopping power in the cold fuel of the NIF capsule. A foil irradiated at the Omega laser at LLE was counted at the LANL low-background counting facility at WIPP. The estimated production rate of {sup 195}Au was just below our experimental sensitivity. We have made several improvements to our counting facility in recent months. These improvements are designed to increase our sensitivity, and include installing two new low-background detectors, and taking steps to reduce noise in the signals.

  3. Low-background spectrometer for the study of fast neutron-induced (n,α) reactions

    NASA Astrophysics Data System (ADS)

    Khriachkov, V. A.; Ketlerov, V. V.; Mitrofanov, V. F.; Semenova, N. N.

    2000-04-01

    An α-particle spectrometer based on an ionization chamber with Frisch grid and a waveform digitizer has been developed for studies of fast neutron-induced (n,α) reactions. The information on the energy of the α-particle and its emission angle can be obtained from the amplitude and rise time of the digitized anode signal. For a situation where both the solid target on the cathode of the ionization chamber and the working gas are the α-particle sources, a new method for the suppression of the neutron-induced background is proposed. The background due to gaseous α-particles was reduced by a factor of 30.

  4. Isospin effects on fragmentation in the asymmetric reactions induced by neutron-rich targets

    NASA Astrophysics Data System (ADS)

    Sharma, Arun

    2016-05-01

    To understand the isospin effects in terms of fragment's yield in the asymmetric reactions induced by neutron-rich targets, we perform a theoretical study using isospin-dependent quantum molecular dynamics (IQMD) model. Simulations are carried out for reactions of 16O+Br80,84,92 and 16O+Ag108,113,122. We envision that fragments's yield in the asymmetric collisions induced by neutron-rich targets is better candidate to study isospin effects via symmetry energy and nucleon-nucleon (nn) cross-sections. Also, pronounced effects of symmetry energy and cross-sections can be found at lower and higher beam energies, respectively.

  5. Active-Interrogation Measurements of Fast Neutrons from Induced Fission in Low-Enriched Uranium

    SciTech Connect

    J. L. Dolan; M. J. Marcath; M. Flaska; S. A. Pozzi; D. L. Chichester; A. Tomanin; P. Peerani

    2014-02-01

    A detection system was designed with MCNPX-PoliMi to measure induced-fission neutrons from U-235 and U-238 using active interrogation. Measurements were then performed with this system at the Joint Research Centre (JRC) in Ispra, Italy on low-enriched uranium samples. Liquid scintillators measured induced fission neutron to characterize the samples in terms of their uranium mass and enrichment. Results are presented to investigate and support the use of organic liquid scintillators with active interrogation techniques to characterize uranium containing materials.

  6. Neutron transfer reactions induced by Li8 on Be9

    NASA Astrophysics Data System (ADS)

    Guimarães, V.; Lichtenthäler, R.; Camargo, O.; Barioni, A.; Assunção, M.; Kolata, J. J.; Amro, H.; Becchetti, F. D.; Jiang, Hao; Aguilera, E. F.; Lizcano, D.; Martines-Quiroz, E.; Garcia, H.

    2007-05-01

    Angular distributions for the elastic scattering of Li8 on Be9 and the neutron transfer reactions Be9(Li8,Li7)Be10 and Be9(Li8,Li9)Be8 were measured with a 27 MeV Li8 radioactive nuclear beam. Spectr- oscopic factors for Li8 ⊗n= Li9 and Li7 ⊗n= Li8 bound systems were obtained from the comparison between the experimental differential cross section and finite-range distorted-wave Born approximation calculations with the code FRESCO. The spectroscopic factors obtained were compared to shell model calculations and to other experimental values from (d,p) reactions. Using the present values for the spectroscopic factor, cross sections for the direct neutron-capture reactions Li7(n,γ)Li8 and Li8(n,γ)Li9 were calculated in the framework of a potential model.

  7. FIGARO: a New Facility for Studying Neutron-Induced Reactions that Produce Gamma Rays

    NASA Astrophysics Data System (ADS)

    Zanini, L.; Haight, R. C.; Devlin, M.; Aprahamian, A.

    2000-04-01

    FIGARO (Fast neutron-Induced GAmma-Ray Observer) was established in 1999 at LANSCE/WNR. This new capability is intended to extend our research into nuclear reactions and nuclear structure using gamma rays as the principal probe. The detector will consist of an array of germanium and NE-213 neutron detectors, operating in coincidence, placed at a distance of about 20 m from the neutron source. The scientific goals of FIGARO include: investigation of nuclear level densities using gamma-ray transitions as an indicator of angular momentum populated in the reaction; investigations of pre-equilibrium reactions; and study of cross sections and neutron emission spectra in (n,n') excitations. A first measurement, with the detection of only gamma-rays, has been performed with a ^59Co sample. By comparison with existing data(T. E. Slusarchyk, ORNL/TM-11404(1989)) we can assess the performance of the detector. Results will be discussed.

  8. Recoil Induced Room Temperature Stable Frenkel Pairs in a-Hafnium Upon Thermal Neutron Capture

    NASA Astrophysics Data System (ADS)

    Butz, Tilman; Das, Satyendra K.; Dey, Chandi C.; Ghoshal, Shamik

    2013-11-01

    Ultrapure hafnium metal (110 ppm zirconium) was neutron activated with a thermal neutron flux of 6:6 · 1012 cm-2s-1 in order to obtain 181Hf for subsequent time differential perturbed angular correlation (TDPAC) experiments using the nuclear probe 181Hf(β-) 181Ta. Apart from the expected nuclear quadrupole interaction (NQI) signal for a hexagonal close-packed (hcp) metal, three further discrete NQIs were observed with a few percent fraction each. The TDPAC spectra were recorded for up to 11 half lives with extreme statistical accuracy. The fitted parameters vary slightly within the temperature range between 248 K and 373 K. The signals corresponding to the three additional sites completely disappear after `annealing' at 453 K for one minute. Based on the symmetry of the additional NQIs and their temperature dependencies, they are tentatively attributed to Frenkel pairs produced by recoil due to the emission of a prompt 5:694 MeV -ray following thermal neutron capture and reported by the nuclear probe in three different positions. These Frenkel pairs are stable up to at least 373 K.

  9. Using Ultracold Neutrons to Characterize Fission Fragment Induced Sputtering

    NASA Astrophysics Data System (ADS)

    Broussard, Leah; Makela, Mark; Morris, Chris

    2015-10-01

    One of the modern challenges in nuclear science and technology is the understanding of the nature of fission fragment damage to material and the resulting ejection of matter as the fragments pass through the surface, with implications to stockpile stewardship and nuclear energy. We have demonstrated a new technique that can be used to characterize the sputtered material with knowledge of the location of the originating fission event. Due to their very high fission cross sections, ultracold neutrons (~100 neV energy) can be used to control the depth at which fission takes place using their energy or the material enrichment. This effort represents one of the first practical applications of ultracold neutrons, which to date have been primarily used to explore questions in fundamental particle physics. We will present results of demonstration measurements including first limits on the total and fission cross sections for 100 neV scale neutrons and the status of the development of this new capability. We gratefully acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program, the G. T. Seaborg Institute, and LANL Science Campaign C1 for this work.

  10. Chromosomal abnormalities in neutron-induced acute myeloid leukemias in CBA/H mice

    SciTech Connect

    Bouffler, S.D.; Meijne, E.I.M.; Huiskamp, R.

    1996-09-01

    Acute myeloid leukemias (AMLs) induced in CBA/H mice by 1 MeV fission neutrons have been examined for chromosomal abnormalities by G-band analysis. In common with X-ray- and {alpha}-particle-induced AMLs in CBA/H mice, more than 90% (16/17) of the myeloid leukemias had chromosome 2 abnormalities, in this case, all interstitial deletions. Chromosome 2 breakpoints were not wholly consistent, but clustering in three specific G-band regions was observed. Very distal (H-region) breakpoints were more common in the neutron AMLs than in X-ray- or {alpha}-particle-induced leukemias. These data indicate that neutron-induced AMLs in CBA/H mice are not characterized by a specific chromosome deletion but that a variety of chromosome 2 deletion types are associated with the disease. Trisomy of chromosome 1 (12.5% AMLs) and aneusomy of chromosomes 6 (31% AMLs) and Y (37.5% AMLs) were noted. While chromatid breakage was observed occasionally in neutron-induced AML, no clear indications of persistent chromosomal instability or high levels of stable chromosomal change were apparent. 19 refs., 1 fig., 1 tab.

  11. Preliminary results of GODIVA-IV prompt burst modeling

    SciTech Connect

    Kimpland, R.

    1996-06-01

    The dynamic computer model developed to simulate GODIVA-IV prompt bursts adequately predicts the magnitude of power bursts. Also, it demonstrates the characteristic features of prompt bursts in metal assemblies, such as the change in shape of power pulses and the ringing of fuel surfaces at the onset of inertial effects. The model will be used to test more sophisticated reactivity feedback coefficients and neutronic-hydrodynamic coupling schemes. It will also be used for a more detailed analysis of inertial effects.

  12. Fission prompt gamma-ray multiplicity distribution measurements and simulations at DANCE

    SciTech Connect

    Chyzh, A; Wu, C Y; Ullmann, J; Jandel, M; Bredeweg, T; Couture, A; Norman, E

    2010-08-24

    The nearly energy independence of the DANCE efficiency and multiplicity response to {gamma} rays makes it possible to measure the prompt {gamma}-ray multiplicity distribution in fission. We demonstrate this unique capability of DANCE through the comparison of {gamma}-ray energy and multiplicity distribution between the measurement and numerical simulation for three radioactive sources {sup 22}Na, {sup 60}Co, and {sup 88}Y. The prospect for measuring the {gamma}-ray multiplicity distribution for both spontaneous and neutron-induced fission is discussed.

  13. Barites - Anomalous xenon from spallation and neutron-induced reactions

    NASA Technical Reports Server (NTRS)

    Srinivasan, B.

    1976-01-01

    Sedimentary barites from South Africa and Western Australia (about 3 billion years old) contain spallogenic Xe isotopes produced by reactions of Ba with nuclear-active particles in cosmic rays. 'Surface residence time' of these samples was calculated from the observed concentrations of spallogenic Xe-126. Comparison of spallogenic ratios of Xe-131/Xe-126 in the two samples provides evidence for the reaction Ba-130(n, gamma) yields Xe-131, which is characterized by a large number of resonances for neutron absorption in the epithermal region. This observation lends additional support to the conclusions already reached regarding the origin of anomalous Xe-131 in lunar samples.

  14. Neutron-induced changes in optical properties of MgAl 2O 4 spinel

    NASA Astrophysics Data System (ADS)

    Ibarra, A.; Garner, F. A.; Hollenberg, G. L.

    1995-03-01

    High purity MgAl 2O 4 spinel specimens irradiated in FFTF-MOTA to very high neutron exposures have been examined by three techniques to determine changes in their optical properties. Significant changes were observed in optical absorption, photoluminescence and radioluminescence, indicating that a variety of radiation-induced defects are present in these specimens.

  15. Continuous versus pulse neutron induced gamma spectroscopy for soil carbon analysis

    Technology Transfer Automated Retrieval System (TEKTRAN)

    Neutron induced gamma spectra analysis (NGA) provides a means of measuring carbon in large soil volumes without destructive sampling. Calibration of the NGA system must account for system background and the interference of other nuclei on the carbon peak at 4.43 MeV. Accounting for these factors pro...

  16. Austenitic stainless steel alloys having improved resistance to fast neutron-induced swelling

    DOEpatents

    Bloom, Everett E.; Stiegler, James O.; Rowcliffe, Arthur F.; Leitnaker, James M.

    1977-03-08

    The present invention is based on the discovery that radiation-induced voids which occur during fast neutron irradiation can be controlled by small but effective additions of titanium and silicon. The void-suppressing effect of these metals in combination is demonstrated and particularly apparent in austenitic stainless steels.

  17. Fast Neutron Induced Autophagy Leads To Necrosis In Glioblastoma Multiforme Cells

    NASA Astrophysics Data System (ADS)

    Yasui, Linda; Gladden, Samantha; Andorf, Christine; Kroc, Thomas

    2011-06-01

    Fast neutrons are highly effective at killing glioblastoma multiforme (GBM), U87 and U251 cells. The mode of cell death was investigated using transmission electron microscopy (TEM) to identify the fraction of irradiated U87 or U251 cells having morphological features of autophagy and/or necrosis. U87 or U251 cells were irradiated with 2 Gy fast neturons or 10 Gy γ rays. A majority of U87 and U251 cells exhibit features of cell death with autophagy after irradiation with either 10 Gy γ rays or 2 Gy fast neutrons. Very few γ irradiated cells had features of necrosis (U87 or U251 cell samples processed for TEM 1 day after 10 Gy γ irradiation). In contrast, a significant increase was observed in necrotic U87 and U251 cells irradiated with fast neutrons. These results show a greater percentage of cells exhibit morphological evidence of necrosis induced by a lower dose of fast neutron irradiation compared to γ irradiation. Also, the evidence of necrosis in fast neutron irradiated U87 and U251 cells occurs in a background of autophagy. Since autophagy is observed before necrosis, autophagy may play a role in signaling programmed necrosis in fast neutron irradiated U87 and U251 cells.

  18. Fast Neutron Induced Autophagy Leads To Necrosis In Glioblastoma Multiforme Cells

    SciTech Connect

    Yasui, Linda; Gladden, Samantha; Andorf, Christine; Kroc, Thomas

    2011-06-01

    Fast neutrons are highly effective at killing glioblastoma multiforme (GBM), U87 and U251 cells. The mode of cell death was investigated using transmission electron microscopy (TEM) to identify the fraction of irradiated U87 or U251 cells having morphological features of autophagy and/or necrosis. U87 or U251 cells were irradiated with 2 Gy fast neturons or 10 Gy {gamma} rays. A majority of U87 and U251 cells exhibit features of cell death with autophagy after irradiation with either 10 Gy {gamma} rays or 2 Gy fast neutrons. Very few {gamma} irradiated cells had features of necrosis (U87 or U251 cell samples processed for TEM 1 day after 10 Gy {gamma} irradiation). In contrast, a significant increase was observed in necrotic U87 and U251 cells irradiated with fast neutrons. These results show a greater percentage of cells exhibit morphological evidence of necrosis induced by a lower dose of fast neutron irradiation compared to {gamma} irradiation. Also, the evidence of necrosis in fast neutron irradiated U87 and U251 cells occurs in a background of autophagy. Since autophagy is observed before necrosis, autophagy may play a role in signaling programmed necrosis in fast neutron irradiated U87 and U251 cells.

  19. Detection of uranium-based nuclear weapons using neutron-induced fission

    SciTech Connect

    Moss, C.E.; Byrd, R.C.; Feldman, W.C.; Auchampaugh, G.F.; Estes, G.P.; Ewing, R.I.; Marlow, K.W.

    1991-12-01

    Although plutonium-based nuclear weapons can usually be detected by their spontaneous emission of neutrons and gammas, the radiation emitted by weapons based entirely on highly-enriched uranium can often be easily shielded. Verification of a treaty that limits the number of such weapons may require an active technique, such as interrogating the suspect assembly with an external neutron source and measuring the number of fission neutrons produced. Difficulties include distinguishing between source and fission neutrons, the variations in yield for different materials and geometries, and the possibility of non-nuclear weapons that may contain significant amounts of fissionable depleted uranium. We describe simple measurements that test the induced-fission technique using an isotopic Am-Li source, an novel energy-sensitive neutron detector, and several small assemblies containing {sup 235}U, {sup 238}U, lead, and polyethylene. In all cases studied, the neutron yields above the source energy are larger for the {sup 235}U assemblies than for assemblies containing only lead or depleted uranium. For more complex geometries, corrections for source transmission may be necessary. The results are promising enough to recommend further experiments and calculations using examples of realistic nuclear and non-nuclear weapons. 5 refs., 11 figs.

  20. Displacement damage effects on CMOS APS image sensors induced by neutron irradiation from a nuclear reactor

    SciTech Connect

    Wang, Zujun Huang, Shaoyan; Liu, Minbo; Xiao, Zhigang; He, Baoping; Yao, Zhibin; Sheng, Jiangkun

    2014-07-15

    The experiments of displacement damage effects on CMOS APS image sensors induced by neutron irradiation from a nuclear reactor are presented. The CMOS APS image sensors are manufactured in the standard 0.35 μm CMOS technology. The flux of neutron beams was about 1.33 × 10{sup 8} n/cm{sup 2}s. The three samples were exposed by 1 MeV neutron equivalent-fluence of 1 × 10{sup 11}, 5 × 10{sup 11}, and 1 × 10{sup 12} n/cm{sup 2}, respectively. The mean dark signal (K{sub D}), dark signal spike, dark signal non-uniformity (DSNU), noise (V{sub N}), saturation output signal voltage (V{sub S}), and dynamic range (DR) versus neutron fluence are investigated. The degradation mechanisms of CMOS APS image sensors are analyzed. The mean dark signal increase due to neutron displacement damage appears to be proportional to displacement damage dose. The dark images from CMOS APS image sensors irradiated by neutrons are presented to investigate the generation of dark signal spike.

  1. Neutron Induced D Breakup in Inertial Confinement Fusion at the Omega Laser Facility

    NASA Astrophysics Data System (ADS)

    Forrest, C. J.; Glebov, V. Yu.; Knauer, J. P.; Radha, P. B.; Regan, S. P.; Sangster, T. C.; Stoeckl, C.; Schroder, W. U.; Frenje, J. A.; Gatu Johnson, M.

    2015-11-01

    High-resolution neutron spectroscopy is used to study the deuteron breakup reaction D(n,n ') np in the thermonuclear environment created in inertial confinement fusion experiments at the Omega Laser Facility. Neutrons with an energy of 14.1 MeV generated in the primary D-T fusion reactions scatter elastically and inelastically off the dense (cryogenic) D-T fuel assembly surrounding the central hot spot at peak fuel compression. These neutrons also induce a breakup of the fuel deuterons. The corresponding breakup cross section is measured relative to elastic n -D and n -T scattering, i.e., simultaneously in the same environment. Apart from astrophysical and technological interest, the neutron-induced deuteron breakup reaction is of interest to the physics of nucleon -nucleon forces. For example, theoretical calculations predict a noticeable influence of nucleonic three-body forces on the magnitude of the breakup cross section. Preliminary results from measurements of the neutron contribution in the 2- to 6-MeV range show reasonable agreement with the published ENDL 2008.2 semi-empirical cross-section. This material is based upon work supported by the Department of Energy National Nuclear Security Administration under Award Number DE-NA0001944.

  2. Use of PuBe source to simulate neutron-induced single event upsets in static RAMS

    SciTech Connect

    Normand, E.; Wert, J.L.; Doherty, W.R.; Oberg, D.L.; Measel, P.R.; Criswell, T.L.

    1988-12-01

    Neutron induced single event upsets were measured in static memory devices using a 10 curie PuBe source. The PuBe source conservatively overestimates the spectrum of fast neutrons emitted by a radioisotope thermoelectric generator (RTG). For the 93L422, the neutron-induced upset rate compared favorably with calculated values derived using the burst generation concept. By accounting for the production of the ionizing particles by the PuBe and RTG neutron spectra, convenient upper bound SEU upset rates for memory devices near an RTG can be derived.

  3. Measurement of gamma-ray production cross sections in neutron-induced reactions for Al and Pb

    SciTech Connect

    Pavlik, A.; Vonach, H.; Hitzenberger, H.; Nelson, R.O.; Haight, R.C.; Wender, S.A.; Young, P.G.; Chadwick, M.B.

    1995-02-01

    The prompt gamma-radiation from the interaction of fast neutrons with aluminum and lead was measured using the white neutron beam of the WNR facility at the Los Alamos National Laboratory. The samples (Al and isotopically enriched {sup 207}Pb and {sup 208}Pb) were positioned at about 20 m or 41 m distance from the neutron production target. The spectra of the emitted gamma-rays were measured with a high-resolution HPGe detector. The incident neutron energy was determined by the time-of-flight method and the neutron fluence was measured with a U fission chamber. From the aluminum gamma-ray spectra excitation functions for prominent gamma-transitions in various residual nuclei (in the range from O to Al) were derived for neutron energies from 3 MeV to 400 MeV. For lead (n,xn{gamma}) reactions were studied for neutron energies up to 200 MeV by analyzing prominent gamma-transitions in the residual nuclei {sup 200,202,204,206,207,208}Pb. The experimental results were compared with nuclear model calculations using the code GNASH. A good overall agreement was obtained without special parameter adjustments.

  4. Characterization of the CRESST detectors by neutron induced nuclear recoils

    NASA Astrophysics Data System (ADS)

    Coppi, C.; Ciemniak, C.; von Feilitzsch, F.; Gütlein, A.; Hagn, H.; Isaila, C.; Jochum, J.; Kimmerle, M.; Lanfranchi, J.-C.; Pfister, S.; Potzel, W.; Rau, W.; Roth, S.; Rottler, K.; Sailer, C.; Scholl, S.; Usherov, I.; Westphal, W.

    CRESST is an experiment for the direct detection of dark matter particles via nuclear recoils. The CRESST detectors, based on CaWO4 scintillating crystals, are able to discriminate γ and β background by simultaneously measuring the light and phonon signals produced by particle interactions. The discrimination of the background is possible because of the different light output (Quenching Factor, QF) for nuclear and electron recoils. In this article a measurement is shown, aimed at the determination of the QFs of the different nuclei (O, Ca, W) of the detector crystal at 40-60 mK using an 11 MeV neutron beam produced at the Maier-Leibnitz-Laboratorium in Garching (MLL).

  5. Neutron-induced latch-up immunity in metal gate CMOS integrated circuits

    SciTech Connect

    Barnes, C.E.; Rollins, J.G.; Hachey, D.

    1987-12-01

    Neutron-induced latch-up immunity has been studied in metal gate CMOS integrated circuits as a function of neutron fluence by measuring both the current gain products (beta product) of parasitic NPN and PNP transistors, and the flash x-ray latch-up thresholds prior to and following irradiation and subsequent stabilization anneal. Correlations between the actual latch-up thresholds and the measured beta products are established for the three part types investigated. These correlations indicate that the measurement of beta products on judiciously chosen parasitic transistors is a viable technique for estimating latch-up susceptibility when the observed margin is substantial.

  6. Fast neutrons-induced apoptosis is Fas-independent in lymphoblastoid cells

    SciTech Connect

    Fischer, Barbara; Benzina, Sami; Jeannequin, Pierre; Dufour, Patrick; Bergerat, Jean-Pierre; Denis, Jean-Marc; Gueulette, John; Bischoff, Pierre L. . E-mail: Pierre.Bischoff@ircad.u-strasbg.fr

    2005-08-26

    We have previously shown that ionizing radiation-induced apoptosis in human lymphoblastoid cells differs according to their p53 status, and that caspase 8-mediated cleavage of BID is involved in the p53-dependent pathway. In the present study, we investigated the role of Fas signaling in caspase 8 activation induced by fast neutrons irradiation in these cells. Fas and FasL expression was assessed by flow cytometry and by immunoblot. We also measured Fas aggregation after irradiation by fluorescence microscopy. We found a decrease of Fas expression after irradiation, but no change in Fas ligand expression. We also showed that, in contrast to the stimulation of Fas by an agonistic antibody, Fas aggregation did not occur after irradiation. Altogether, our data strongly suggest that fast neutrons induced-apoptosis is Fas-independent, even in p53-dependent apoptosis.

  7. Signatures of field induced spin polarization of neutron star matter in seismic vibrations of paramagnetic neutron star

    NASA Astrophysics Data System (ADS)

    Bastrukov, S. I.; Yang, J.; Podgainy, D. V.; Weber, F.

    2003-04-01

    A macroscopic model of the dissipative magneto-elastic dynamics of viscous spin polarized nuclear matter is discussed in the context of seismic activity of a paramagnetic neutron star. The source of the magnetic field of such a star is attributed to Pauli paramagnetism of baryon matter promoted by a seed magnetic field frozen into the star in the process of gravitational collapse of a massive progenitor. Particular attention is given to the effect of shear viscosity of incompressible stellar material on the timing of non-radial torsional magneto-elastic pulsations of the star triggered by starquakes. By accentuating the fact that this kind of vibration is unique to the seismology of a paramagnetic neutron star we show that the high-frequency modes decay faster than the low-frequency modes. The obtained analytic expressions for the period and relaxation time of this mode, in which the magnetic susceptibility and viscosity enter as input parameters, are then quantified by numerical estimates for these parameters taken from early and current works on transport coefficients of dense matter. It is found that the effect of viscosity is crucial for the lifetime of magneto-torsion vibrations but it does not appreciably affect the periods of this seismic mode which fall in the realm of periods of pulsed emission of soft gamma-ray repeaters and anomalous x-ray pulsars - young super-magnetized neutron stars, radiating, according to the magnetar model, at the expense of the magnetic energy release. Finally, we present arguments that the long periodic pulsed emission of these stars in a quiescent regime of radiation can be interpreted as a manifestation of weakly damped seismic magneto-torsion vibrations exhibiting the field induced spin polarization of baryon matter.

  8. A measurement of the muon-induced neutron yield in lead at a depth of 2850 m water equivalent

    SciTech Connect

    Reichhart, L.; Ghag, C.; Lindote, A.; Chepel, V.; DeViveiros, L.; Lopes, M. I.; Neves, F.; Pinto da Cunha, J.; Silva, C.; Solovov, V. N.; Akimov, D. Yu.; Belov, V. A.; Burenkov, A. A.; Kobyakin, A. S.; Kovalenko, A. G.; Stekhanov, V. N.; Araújo, H. M.; Bewick, A.; Currie, A.; Horn, M.; and others

    2013-08-08

    We present results from the measurement of the neutron production rate in lead by high energy cosmic-ray muons at a depth of 2850 m water equivalent (mean muon energy of 260 GeV). A tonne-scale highly segmented plastic scintillator detector was utilised to detect both the energy depositions from the traversing muons as well as the delayed radiative capture signals of the induced neutrons. Complementary Monte Carlo simulations reproduce well the distributions of muons and detected muon-induced neutrons. Absolute agreement between simulation and data is of the order of 25%. By comparing the measured and simulated neutron capture rates a neutron yield in pure lead of (5.78{sub −0.28}{sup +0.21})×10{sup −3} neutrons/muon/(g/cm{sup 2}) has been obtained.

  9. Neutron-induced reactions on AlF3 studied using the optical model

    NASA Astrophysics Data System (ADS)

    Ma, Chun-Wang; Lv, Cui-Juan; Zhang, Guo-Qiang; Wang, Hong-Wei; Zuo, Jia-Xu

    2015-08-01

    Neutron-induced reactions on 27Al and 19F nuclei are investigated using the optical model implemented in the TALYS 1.4 toolkit. Incident neutron energies in a wide range from 0.1 keV to 30 MeV are calculated. The cross sections for the main channels (n, np), (n, p), (n, α), (n, 2n), and (n, γ) and the total reaction cross section (n, tot) of the reactions are obtained. When the default parameters in TALYS 1.4 are adopted, the calculated results agree with the measured results. Based on the calculated results for the n + 27Al and n + 19F reactions, the results of the n + 27Al19F reactions are predicted. These results are useful both for the design of thorium-based molten salt reactors and for neutron activation analysis techniques.

  10. In-situ measurement of the rate of U-235 fission induced by lunar neutrons

    NASA Technical Reports Server (NTRS)

    Woolum, D. S.; Burnett, D. S.

    1974-01-01

    The depth profile of the neutron-induced fission rate of U-235 was directly measured to a depth of 350 g/sq cm by the Apollo 17 Lunar Neutron Probe Experiment. The fission rate rises sharply from the surface to a broad maximum from 110 to 160 g/sq cm and drops off at greater depths. The shape of the theoretical depth profile of Lingenfelter et al (1972) fits the measured capture rates well at all depths. The absolute magnitude of the experimental fission rates are (11 plus or minus 17)% lower than those calculated theoretically. The excellent agreement between theory and experiment implies that conclusions drawn previously by interpreting lunar sample data with the theoretical capture rates will not require revision. In particular, lunar surface processes, rather than uncertainties in the capture rates, are required to explain the relatively low neutron fluences observed for surface soil samples compared to the fluences expected for a uniformly mixed regolith.

  11. Determination of the 243,246,248Cm thermal neutron induced fission cross sections

    NASA Astrophysics Data System (ADS)

    Serot, O.; Wagemans, C.; Vermote, S.; Heyse, J.; Soldner, T.; Geltenbort, P.

    2005-11-01

    The minor actinide waste produced in nuclear power plants contains various Cm-isotopes, and transmutation scenarios require improved fission cross section data. The available thermal neutron induced fission cross section data for 243Cm, 246Cm and 248Cm are not very accurate, so new cross section measurements have been performed at the high flux reactor of the ILL in Grenoble (France) under better experimental conditions (highly enriched samples, very intense and clean neutron beam). The measurements were performed at a neutron energy of 5.38 meV, yielding fission cross section values of (1240±28)b for 243Cm, (25±47)mb for 246Cm and (685±84)mb for 248Cm. From these results, thermal fission cross section values of (572±14)b; (12±25)mb and (316±43)mb have been deduced for 243Cm, 246Cm and 248Cm, respectively.

  12. Analysis of the Nuclear Structure of 186 Re Using Neutron-Induced Reactions

    NASA Astrophysics Data System (ADS)

    Matters, David; McClory, John; Carroll, James; Chiara, Chris; Fotiades, Nikolaos; Devlin, Matt; Nelson, Ron O.

    2015-04-01

    Evaluated nuclear structure data for 186 Re identifies the majority of spin-parity assignments as tentative, with approximate values associated with the energies of several levels and transitions. In particular, the absence of known transitions that feed the Jπ =8+ isomer motivates their discovery, which would have astrophysical implications and a potential application in the development of an isomer power source. Using the GErmanium Array for Neutron Induced Excitations (GEANIE) spectrometer at the Los Alamos Neutron Science Center (LANSCE) Weapons Neutron Research (WNR) facility, the (n,2n γ) and (n,n' γ) reactions in a 99.52% enriched 187 Re target were used to measure γ-ray excitation functions in 186 Re and 187 Re, respectively. A preliminary analysis of the data obtained from the experiment reveals several new transitions in 186 Re and 187 Re.

  13. A New Facility for High-Energy Neutron-Induced Fission Studies

    SciTech Connect

    Prokofiev, A.; Carlsson, M.; Einarsson, L.; Haag, N.; Pomp, S.; Bergenwall, B.; Blomgren, J.; Hildebrand, A.; Johansson, C.; Mermod, P.; Oesterlund, M.; Tippawan, U.; Dangtip, S.

    2005-05-24

    A new facility is constructed for measurements of neutron-induced fission cross sections in the 20-180 MeV energy region versus the np scattering cross section, which is adopted as the primary neutron standard. The advantage of the experiment compared to earlier studies is that the fission-fragment detection and the neutron-flux measurement via np scattering are performed simultaneously and at the same position in the beam, and, therefore, many sources of systematic errors cancel out. Further reduction of systematic errors is achieved due to 'embedded' determination of effective solid angle of particle detectors using {alpha}-particles from the radioactive decay of the target nuclei. The performance of the facility is illustrated by first data obtained for angular distributions of fission fragments in the 238U(n,f) reaction.

  14. Neutron-induced gamma-ray spectroscopy: simulations for chemical mapping of planetary surfaces

    SciTech Connect

    Brueckner, J.; Waenke, H.; Reedy, R.C.

    1986-01-01

    Cosmic rays interact with the surface of a planetary body and produce a cascade of secondary particles, such as neutrons. Neutron-induced scattering and capture reactions play an important role in the production of discrete gamma-ray lines that can be measured by a gamma-ray spectrometer on board of an orbiting spacecraft. These data can be used to determine the concentration of many elements in the surface of a planetary body, which provides clues to its bulk composition and in turn to its origin and evolution. To investigate the gamma rays made by neutron interactions, thin targets were irradiated with neutrons having energies from 14 MeV to 0.025 eV. By means of foil activation technique the ratio of epithermal to thermal neutrons was determined to be similar to that in the Moon. Gamma rays emitted by the targets and the surrounding material were detected by a high-resolution germanium detector in the energy range of 0.1 to 8 MeV. Most of the gamma-ray lines that are expected to be used for planetary gamma-ray spectroscopy were found in the recorded spectra and the principal lines in these spectra are presented. 58 refs., 7 figs., 9 tabs.

  15. Measurements and simulations of the cosmic-ray-induced neutron background

    NASA Astrophysics Data System (ADS)

    Becchetti, M. F.; Flaska, M.; Clarke, S. D.; Pozzi, S. A.

    2015-03-01

    The cosmic-ray-induced neutron background at ground level has been measured and simulated in conjunction with EJ-309 organic liquid scintillators with an approximate deposited energy range of 0.5-6 MeV. Specifically, the pulse height distributions, net neutron count rates, and angular dependences were obtained. The simulations were carried out using the Monte Carlo transport code MCNPX-PoliMi combined with the (Cosmic-Ray Shower Generator) CRY source subroutine that returns secondary particles produced by cosmic rays. A scaling formula from literature was also implemented in the simulation. The angular dependence of the neutron count rate was measured by collimating the liquid scintillator with polyethylene to attain 18° angular resolution from 0° downwards to 72° horizontally. The neutron count rate was measured to be 23.10±1.69 h-1 sr-1 at 0°, and 7.20±0.78 h-1 sr-1 at 72°. The simulations and measurements compare well and show similar cosine anisotropy for the angular distribution. The study thus shows that the neutron background response in detector systems can be efficiently and accurately simulated using the procedures described.

  16. Predicted neutron yield and radioactivity for laser-induced (p,n) reactions in LiF

    SciTech Connect

    Swift, D C; McNaney, J M

    2009-01-30

    Design calculations are presented for a pulsed neutron source comprising polychromatic protons accelerated from a metal foil by a short-pulse laser, and a LiF converter in which (p,n) reactions occur. Although the proton pulse is directional, neutrons are predicted to be emitted relatively isotropically. The neutron spectrum was predicted to be similar to the proton spectrum, but with more neutrons of low energy in the opposite direction to the incident protons. The angular dependence of spectrum and intensity was predicted. The (p,n) reactions generate unstable nuclei which decay predominantly by positron emission to the original {sup 7}Li and {sup 19}F isotopes. For the initial planned experiments using a converter 1mm thick, we predict that 0.1% of the protons will undergo a (p,n) reaction, producing 10{sup 9} neutrons. Ignoring the unreacted protons, neutrons, and prompt gamma emission as excited nuclear states decay, residual positron radioactivity (and production of pairs of 511 keV annihilation photons) is initially 4.2MBq decaying with a half-life of 17.22 s for 6 mins ({sup 19}Ne decays), then 135Bq decaying with a half-life of 53.22 days ({sup 7}Be decays).

  17. Fast-neutron spectroscopy studies using induced-proton tracks in PADC track detectors

    NASA Astrophysics Data System (ADS)

    El-Sersy, A. R.; Eman, S. A.

    2010-06-01

    In this work, a simple and adequate method for fast-neutron spectroscopy is proposed. This method was performed by free-in-air fast-neutron irradiation of CR-39 Nuclear Track Detectors (NTD) using an Am-Be source. Detectors were then chemically etched to remove few layers up to a thickness of 6.25 μm. By using an automatic image analyzer system for studying the registration of the induced-proton tracks in the NTD, the obtained data were analyzed via two tracks shapes. In the first one, the elliptical tracks were eliminated from the calculation and only the circular ones were considered in developing the response function. In the second method all registered tracks were considered and the corresponding response function was obtained. The rate of energy loss of the protons as a function of V[(d E/d X) - V] was calculated using the Monte Carlo simulation. The induced-proton energy was extracted from the corresponding d E/d X in NTD using a computer program based on the Bethe-Bloch function. The energy of the incident particles was up to few hundred MeV/nucleon. The energy of the interacting neutrons was then estimated by means of the extracted induced-proton energies and the scattering angle. It was found that the present resulting energy distribution of the fast-neutron spectrum from the Am-Be source was similar to that given in the literature where an average neutron energy of 4.6MeV was obtained.

  18. DNA damage induced by boron neutron capture therapy is partially repaired by DNA ligase IV.

    PubMed

    Kondo, Natsuko; Sakurai, Yoshinori; Hirota, Yuki; Tanaka, Hiroki; Watanabe, Tsubasa; Nakagawa, Yosuke; Narabayashi, Masaru; Kinashi, Yuko; Miyatake, Shin-ichi; Hasegawa, Masatoshi; Suzuki, Minoru; Masunaga, Shin-ichiro; Ohnishi, Takeo; Ono, Koji

    2016-03-01

    Boron neutron capture therapy (BNCT) is a particle radiation therapy that involves the use of a thermal or epithermal neutron beam in combination with a boron ((10)B)-containing compound that specifically accumulates in tumor. (10)B captures neutrons and the resultant fission reaction produces an alpha ((4)He) particle and a recoiled lithium nucleus ((7)Li). These particles have the characteristics of high linear energy transfer (LET) radiation and therefore have marked biological effects. High-LET radiation is a potent inducer of DNA damage, specifically of DNA double-strand breaks (DSBs). The aim of the present study was to clarify the role of DNA ligase IV, a key player in the non-homologous end-joining repair pathway, in the repair of BNCT-induced DSBs. We analyzed the cellular sensitivity of the mouse embryonic fibroblast cell lines Lig4-/- p53-/- and Lig4+/+ p53-/- to irradiation using a thermal neutron beam in the presence or absence of (10)B-para-boronophenylalanine (BPA). The Lig4-/- p53-/- cell line had a higher sensitivity than the Lig4+/+ p53-/-cell line to irradiation with the beam alone or the beam in combination with BPA. In BNCT (with BPA), both cell lines exhibited a reduction of the 50 % survival dose (D 50) by a factor of 1.4 compared with gamma-ray and neutron mixed beam (without BPA). Although it was found that (10)B uptake was higher in the Lig4+/+ p53-/- than in the Lig4-/- p53-/- cell line, the latter showed higher sensitivity than the former, even when compared at an equivalent (10)B concentration. These results indicate that BNCT-induced DNA damage is partially repaired using DNA ligase IV. PMID:26573366

  19. Reducing Uncertainties in Neutron-Induced Fission Cross Sections Using a Time Projection Chamber

    NASA Astrophysics Data System (ADS)

    Manning, Brett; Niffte Collaboration

    2015-10-01

    Neutron-induced fission cross sections for actinides have long been of great interest for nuclear energy and stockpile stewardship. Traditionally, measurements were performed using fission chambers which provided limited information about the detected fission events. For the case of 239Pu(n,f), sensitivity studies have shown a need for more precise measurements. Recently the Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) has developed the fission Time Projection Chamber (fissionTPC) to measure fission cross sections to better than 1% uncertainty by providing 3D tracking of fission fragments. The fissionTPC collected data to calculate the 239Pu(n,f) cross section at the Weapons Neutron Research facility at the Los Alamos Neutron Science Center during the 2014 run cycle. Preliminary analysis has been focused on studying particle identification and target and beam non-uniformities to reduce the uncertainty on the cross section. Additionally, the collaboration is investigating other systematic errors that could not be well studied with a traditional fission chamber. LA-UR-15-24906.

  20. Observation of Gravitationally Induced Vertical Striation of Polarized Ultracold Neutrons by Spin-Echo Spectroscopy

    NASA Astrophysics Data System (ADS)

    Afach, S.; Ayres, N. J.; Ban, G.; Bison, G.; Bodek, K.; Chowdhuri, Z.; Daum, M.; Fertl, M.; Franke, B.; Griffith, W. C.; Grujić, Z. D.; Harris, P. G.; Heil, W.; Hélaine, V.; Kasprzak, M.; Kermaidic, Y.; Kirch, K.; Knowles, P.; Koch, H.-C.; Komposch, S.; Kozela, A.; Krempel, J.; Lauss, B.; Lefort, T.; Lemière, Y.; Mtchedlishvili, A.; Musgrave, M.; Naviliat-Cuncic, O.; Pendlebury, J. M.; Piegsa, F. M.; Pignol, G.; Plonka-Spehr, C.; Prashanth, P. N.; Quéméner, G.; Rawlik, M.; Rebreyend, D.; Ries, D.; Roccia, S.; Rozpedzik, D.; Schmidt-Wellenburg, P.; Severijns, N.; Thorne, J. A.; Weis, A.; Wursten, E.; Wyszynski, G.; Zejma, J.; Zenner, J.; Zsigmond, G.

    2015-10-01

    We describe a spin-echo method for ultracold neutrons (UCNs) confined in a precession chamber and exposed to a |B0|=1 μ T magnetic field. We have demonstrated that the analysis of UCN spin-echo resonance signals in combination with knowledge of the ambient magnetic field provides an excellent method by which to reconstruct the energy spectrum of a confined ensemble of neutrons. The method takes advantage of the relative dephasing of spins arising from a gravitationally induced striation of stored UCNs of different energies, and also permits an improved determination of the vertical magnetic-field gradient with an exceptional accuracy of 1.1 pT /cm . This novel combination of a well-known nuclear resonance method and gravitationally induced vertical striation is unique in the realm of nuclear and particle physics and should prove to be invaluable for the assessment of systematic effects in precision experiments such as searches for an electric dipole moment of the neutron or the measurement of the neutron lifetime.

  1. Observation of Gravitationally Induced Vertical Striation of Polarized Ultracold Neutrons by Spin-Echo Spectroscopy.

    PubMed

    Afach, S; Ayres, N J; Ban, G; Bison, G; Bodek, K; Chowdhuri, Z; Daum, M; Fertl, M; Franke, B; Griffith, W C; Grujić, Z D; Harris, P G; Heil, W; Hélaine, V; Kasprzak, M; Kermaidic, Y; Kirch, K; Knowles, P; Koch, H-C; Komposch, S; Kozela, A; Krempel, J; Lauss, B; Lefort, T; Lemière, Y; Mtchedlishvili, A; Musgrave, M; Naviliat-Cuncic, O; Pendlebury, J M; Piegsa, F M; Pignol, G; Plonka-Spehr, C; Prashanth, P N; Quéméner, G; Rawlik, M; Rebreyend, D; Ries, D; Roccia, S; Rozpedzik, D; Schmidt-Wellenburg, P; Severijns, N; Thorne, J A; Weis, A; Wursten, E; Wyszynski, G; Zejma, J; Zenner, J; Zsigmond, G

    2015-10-16

    We describe a spin-echo method for ultracold neutrons (UCNs) confined in a precession chamber and exposed to a |B0|=1  μT magnetic field. We have demonstrated that the analysis of UCN spin-echo resonance signals in combination with knowledge of the ambient magnetic field provides an excellent method by which to reconstruct the energy spectrum of a confined ensemble of neutrons. The method takes advantage of the relative dephasing of spins arising from a gravitationally induced striation of stored UCNs of different energies, and also permits an improved determination of the vertical magnetic-field gradient with an exceptional accuracy of 1.1  pT/cm. This novel combination of a well-known nuclear resonance method and gravitationally induced vertical striation is unique in the realm of nuclear and particle physics and should prove to be invaluable for the assessment of systematic effects in precision experiments such as searches for an electric dipole moment of the neutron or the measurement of the neutron lifetime. PMID:26550870

  2. Super_Prompt Crit excursions in Sph Geometry

    Energy Science and Technology Software Center (ESTSC)

    2000-03-17

    AX-TNT solves (a) the coupled hydrodynamic, thermodynamical neutronic equations which describe a spherical, super prompt critical reactor system during an excursion. (b) the coupled equations of motion, and ideal gas equation of state for the detonation of a spherical charge in a gas.

  3. Detection of special nuclear material by observation of delayed neutrons with a novel fast neutron composite detector

    NASA Astrophysics Data System (ADS)

    Mayer, Michael; Nattress, Jason; Barhoumi Meddeb, Amira; Foster, Albert; Trivelpiece, Cory; Rose, Paul; Erickson, Anna; Ounaies, Zoubeida; Jovanovic, Igor

    2015-10-01

    Detection of shielded special nuclear material is crucial to countering nuclear terrorism and proliferation, but its detection is challenging. By observing the emission of delayed neutrons, which is a unique signature of nuclear fission, the presence of nuclear material can be inferred. We report on the observation of delayed neutrons from natural uranium by using monoenergetic photons and neutrons to induce fission. An interrogating beam of 4.4 MeV and 15.1 MeV gamma-rays and neutrons was produced using the 11B(d,n-γ)12C reaction and used to probe different targets. Neutron detectors with complementary Cherenkov detectors then discriminate material undergoing fission. A Li-doped glass-polymer composite neutron detector was used, which displays excellent n/ γ discrimination even at low energies, to observe delayed neutrons from uranium fission. Delayed neutrons have relatively low energies (~0.5 MeV) compared to prompt neutrons, which makes them difficult to detect using recoil-based detectors. Neutrons were counted and timed after the beam was turned off to observe the characteristic decaying time profile of delayed neutrons. The expected decay of neutron emission rate is in agreement with the common parametrization into six delayed neutron groups.

  4. Nuclear Astrophysics and Neutron Induced Reactions: Quasi-Free Reactions and RIBs

    SciTech Connect

    Cherubini, S.; Spitaleri, C.; Crucilla, V.; Gulino, M.; La Cognata, M.; Lamia, L.; Pizzone, R. G.; Puglia, S.; Rapisarda, G. G.; Romano, S.; Sergi, M. L.; Coc, A.; Kubono, S.; Binh, D. N.; Hayakawa, S.; Wakabayashi, Y.; Yamaguchi, H.; Burjan, V.; Kroha, V.; De Sereville, N.

    2010-08-12

    The use of quasi-free reactions in studying nuclear reactions between charged particles of astrophysical interest has received much attention over the last two decades. The Trojan Horse Method is based on this approach and it has been used to study a number of reactions relevant for Nuclear Astrophysics. Recently we applied this method to the study of nuclear reactions that involve radioactive species, namely to the study of the {sup 18}F+p{yields}{sup 15}O+{alpha} process at temperatures corresponding to the energies available in the classical novae scenario. Quasi-free reactions can also be exploited to study processes induced by neutrons. This technique is particularly interesting when applied to reaction induced by neutrons on unstable short-lived nuclei. Such processes are very important in the nucleosynthesis of elements in the sand r-processes scenarios and this technique can give hints for solving key questions in nuclear astrophysics where direct measurements are practically impossible.

  5. 231Pa and 233Pa Neutron-Induced Fission Data Analysis

    SciTech Connect

    Maslov, V.M.; Tetereva, N.A.; Baba, M.; Hasegawa, A.; Kornilov, N.V.; Kagalenko, A.B.

    2005-05-24

    The 231Pa and 233Pa neutron-induced fission cross-section database is analyzed within the Hauser-Feshbach approach. The consistency of neutron-induced fission cross-section data and data extracted from transfer reactions is investigated. The fission probabilities of Pa, fissioning in 231,233Pa(n,nf) reactions, are defined by fitting (3He,d) or (3He,t) transfer-reaction data. The present estimate of the 233Pa(n,f) fission cross section above the emissive fission threshold is supported by smooth level-density parameter systematics, validated in the case of the 231Pa(n,f) data description up to En =20 MeV.

  6. Prompting Strategies for Introducing Opera.

    ERIC Educational Resources Information Center

    Beck, Charles R.

    2002-01-01

    Describes how to introduce opera to students through the use of prompting strategies. Explains that these strategies encourage active participation by students and help to improve listening skills. Focuses on prompting strategies, such as matching characters to songs, identifying, and sequencing songs. (CMK)

  7. Modeled Neutron Induced Nuclear Reaction Cross Sections for Radiochemistry in the region of Iriduim and Gold

    SciTech Connect

    Hoffman, R D; Dietrich, F S; Kelley, K; Escher, J; Bauer, R; Mustafa, M

    2008-02-26

    We have developed a set of modeled nuclear reaction cross sections for use in radiochemical diagnostics. Systematics for the input parameters required by the Hauser-Feshbach statistical model were developed and used to calculate neutron induced nuclear reaction cross sections for targets ranging from osmium (Z = 76) to gold (Z = 79). Of particular interest are the cross sections on Ir and Au including reactions on isomeric targets.

  8. Welding-induced microstructure in austenitic stainless steels before and after neutron irradiation

    NASA Astrophysics Data System (ADS)

    Stoenescu, R.; Schäublin, R.; Gavillet, D.; Baluc, N.

    2007-02-01

    The effects of neutron irradiation on the microstructure of welded joints made of austenitic stainless steels have been investigated. The materials were welded AISI 304 and AISI 347, so-called test weld materials, and irradiated with neutrons at 300 °C to 0.3 and 1.0 dpa. In addition, an AISI 304 type from a decommissioned pressurised water reactor, so-called in-service material, which had accumulated a maximum dose of 0.35 dpa at about 300 °C, was investigated. The microstructure of heat-affected zones and base materials was analysed before and after irradiation, using transmission electron microscopy. Neutron diffraction was performed for internal stress measurements. It was found that the heat-affected zone contains, relative to the base material, a higher dislocation density, which relates well to a higher residual stress level and, after irradiation, a higher irradiation-induced defect density. In both materials, the irradiation-induced defects are of the same type, consisting in black dots and Frank dislocation loops. Careful analysis of the irradiation-induced defect contrast was performed and it is explained why no stacking fault tetrahedra could be identified.

  9. Simulation of synergistic effects on lateral PNP bipolar transistors induced by neutron and gamma irradiation

    NASA Astrophysics Data System (ADS)

    Wang, Chenhui; Bai, Xiaoyan; Chen, Wei; Yang, Shanchao; Liu, Yan; Jin, Xiaoming; Ding, Lili

    2015-10-01

    With semiconductor device simulation software TCAD, numerical simulations of ionizing/displacement synergistic effects on 6 kinds of lateral PNP bipolar transistors induced by the mixed irradiation of neutron and gamma are carried out by means of changing the minority carrier lifetimes, adding charged traps to the oxide layer and increasing the surface recombination velocity in Si/SiO2 interface. The results indicate that ionizing/displacement synergistic effects on the lateral PNP bipolar transistors are not a simple sum of total ionizing dose effects and displacement effects, and total ionizing dose effects can enhance neutron displacement damages, leading to greater gain degradation. The physical mechanisms of ionizing/displacement synergistic effects are analyzed based on the results. The positive charge in the oxide layer and Si/SiO2 interface traps induced by gamma irradiation can enhance the recombination processes of carriers in the bulk defects induced by neutron irradiation, and this is the main cause of ionizing/displacement synergistic effects on the lateral PNP bipolar transistors.

  10. Small punch test evaluation of neutron-irradiation-induced embrittlement of a Cr-Mo low-alloy steel

    SciTech Connect

    Song, S.-H. . E-mail: shsonguk@yahoo.co.uk; Faulkner, R.G.; Flewitt, P.E.J.; Marmy, P.; Weng, L.-Q.

    2004-09-15

    Neutron-irradiation-induced embrittlement of a 2.25Cr1Mo steel is investigated by means of small punch testing along with scanning electron microscopy. There is an apparent irradiation-induced embrittlement effect after the steel is irradiated at about 400 deg. C for 86 days with a neutron dose rate of 1.75x10{sup -8} dpa/s. The embrittlement is mainly nonhardening embrittlement caused by impurity grain boundary segregation.

  11. Measurement of cosmic-ray muons and muon-induced neutrons in the Aberdeen Tunnel Underground Laboratory

    NASA Astrophysics Data System (ADS)

    Blyth, S. C.; Chan, Y. L.; Chen, X. C.; Chu, M. C.; Cui, K. X.; Hahn, R. L.; Ho, T. H.; Hsiung, Y. B.; Hu, B. Z.; Kwan, K. K.; Kwok, M. W.; Kwok, T.; Lau, Y. P.; Leung, J. K. C.; Leung, K. Y.; Lin, G. L.; Lin, Y. C.; Luk, K. B.; Luk, W. H.; Ngai, H. Y.; Ngan, S. Y.; Pun, C. S. J.; Shih, K.; Tam, Y. H.; Tsang, R. H. M.; Wang, C. H.; Wong, C. M.; Wong, H. L. H.; Wong, K. K.; Yeh, M.; Zhang, B. J.; Aberdeen Tunnel Experiment Collaboration

    2016-04-01

    We have measured the muon flux and production rate of muon-induced neutrons at a depth of 611 m water equivalent. Our apparatus comprises three layers of crossed plastic scintillator hodoscopes for tracking the incident cosmic-ray muons and 760 L of a gadolinium-doped liquid scintillator for producing and detecting neutrons. The vertical muon intensity was measured to be Iμ=(5.7 ±0.6 )×10-6 cm-2 s-1 sr-1 . The yield of muon-induced neutrons in the liquid scintillator was determined to be Yn=(1.19 ±0.08 (stat)±0.21 (syst))×10-4 neutrons /(μ .g .cm-2 ) . A fit to the recently measured neutron yields at different depths gave a mean muon energy dependence of ⟨Eμ⟩ 0.76 ±0.03 for liquid-scintillator targets.

  12. Measurement of cosmic-ray muons and muon-induced neutrons in the Aberdeen Tunnel Underground Laboratory

    DOE PAGESBeta

    Yeh, M.; Chan, Y. L.; Chen, X. C.; Chu, M. C.; Cui, K. X.; Hahn, R. L.; Ho, T. H.; Hsiung, Y. B.; Hu, B. Z.; Kwan, K. K.; et al

    2016-04-07

    In this study, we have measured the muon flux and production rate of muon-induced neutrons at a depth of 611 m water equivalent. Our apparatus comprises three layers of crossed plastic scintillator hodoscopes for tracking the incident cosmic-ray muons and 760 L of a gadolinium-doped liquid scintillator for producing and detecting neutrons. The vertical muon intensity was measured to be Iμ = (5.7±0.6)×10–6 cm–2 s–1 sr–1. The yield of muon-induced neutrons in the liquid scintillator was determined to be Yn = (1.19 ± 0.08(stat) ± 0.21(syst)) × 10–4 neutrons/(μ•g•cm–2). A fit to the recently measured neutron yields at different depthsmore » gave a mean muon energy dependence of < Eμ >0.76±0.03 for liquid-scintillator targets.« less

  13. QED vacuum fluctuations and induced electric dipole moment of the neutron

    SciTech Connect

    Dominguez, C. A.; Falomir, H.; Ipinza, M.; Loewe, M.; Kohler, S.; Rojas, J. C.

    2009-08-01

    Quantum fluctuations in the QED vacuum generate nonlinear effects, such as peculiar induced electromagnetic fields. In particular, we show here that an electrically neutral particle, possessing a magnetic dipole moment, develops an induced electric dipole-type moment with unusual angular dependence, when immersed in a quasistatic, constant external electric field. The calculation of this effect is done in the framework of the Euler-Heisenberg effective QED Lagrangian, corresponding to the weak field asymptotic expansion of the effective action to one-loop order. It is argued that the neutron might be a good candidate to probe this signal of nonlinearity in QED.

  14. Terahertz, X-ray and neutron computed tomography of an Eighteenth Dynasty Egyptian sealed pottery

    NASA Astrophysics Data System (ADS)

    Abraham, E.; Bessou, M.; Ziéglé, A.; Hervé, M.-C.; Szentmiklósi, L.; Kasztovszky, Z. S.; Kis, Z.; Menu, M.

    2014-09-01

    An Eighteenth Dynasty Egyptian sealed pottery stored at the Museum of Aquitaine (Bordeaux, France) has been investigated using terahertz radiation, X-rays and neutrons. THz computed tomography revealed nondestructively the presence of content, whereas X-rays and neutrons analyzed more precisely the fabrication process and conservation of the pottery together with the nature of this content owing to higher spatial resolution and contrast. With neutron tomography, we determined the method used to seal the jar as well as the finer structure of the inner content. Neutron-induced prompt gamma spectroscopy was finally applied to measure the elemental composition of the content, which is supposed to consist of dried germinated seeds.

  15. Laser-induced fluorescence measurements of NCN in low-pressure CH{sub 4}/O{sub 2}/N{sub 2} flames and its role in prompt NO formation

    SciTech Connect

    Sutton, Jeffrey A.; Williams, Bradley A.; Fleming, James W.

    2008-05-15

    NCN profiles were measured for five rich and lean premixed, low-pressure methane flames using laser-induced fluorescence (LIF). A semiquantitative determination of the NCN mole fractions as a function of spatial height above the burner is made by calibrating the NCN LIF signals using highly accurate OH LIF measurements in an adjacent spectral region. The resulting calibration yields an uncertainty estimate of a factor of 3 for the absolute values, but only {+-}25% for the relative NCN profiles. For all flame conditions, the NCN profiles occur immediately downstream of previously measured CH profiles. In addition, high correlations are found between the peak CH and peak NCN concentrations and the peak NCN and postflame NO concentrations over all equivalence ratios. These observations are consistent with NCN being the primary product channel from the CH + N{sub 2} reaction and the initial intermediate in the prompt NO formation. This is the first mechanistic study in hydrocarbon flames that provides such experimental evidence. The experimental profiles are compared to numerical calculations using modified versions of two well-established hydrocarbon kinetic mechanisms. Reasonable agreement between the calculations and experiment is found for NCN profile shape, location of peak NCN concentrations, and absolute mole fractions. However, the dependence on stoichiometry of the peak NCN concentration is overestimated. Further work is required on NCN kinetics for modeling prompt NO in laminar premixed flames. (author)

  16. Measurement and modeling of muon-induced neutrons in LSM in application for direct dark matter searches

    SciTech Connect

    Kozlov, Valentin; Collaboration: EDELWEISS Collaboration

    2013-08-08

    Due to a very low event rate expected in direct dark matter search experiments, a good understanding of every background component is crucial. Muon-induced neutrons constitute a prominent background, since neutrons lead to nuclear recoils and thus can mimic a potential dark matter signal. EDELWEISS is a Ge-bolometer experiment searching for WIMP dark matter. It is located in the Laboratoire Souterrain de Modane (LSM, France). We have measured muon-induced neutrons by means of a neutron counter based on Gd-loaded liquid scintillator. Studies of muon-induced neutrons are presented and include development of the appropriate MC model based on Geant4 and analysis of a 1000-days measurement campaign in LSM. We find a good agreement between measured rates of muon-induced neutrons and those predicted by the developed model with full event topology. The impact of the neutron background on current EDELWEISS data-taking as well as for next generation experiments such as EURECA is briefly discussed.

  17. Simulation of neutron-induced damage in tungsten by irradiation with energetic self-ions

    NASA Astrophysics Data System (ADS)

    Ogorodnikova, O. V.; Gann, V.

    2015-05-01

    A direct comparison of the deuterium (D) decoration of radiation-induced damage in polycrystalline tungsten irradiated with self-ions [present work] and neutrons in the high-flux isotope reactor (HFIR) (Hatano et al., 2013) shows a reasonably good agreement at least up to 0.3 displacement per atom indicating that MeV heavy ions can be a good proxy to simulate neutron-produced damage at room temperature and low dpa. The coefficient of similarity between two kinds of irradiation was obtained experimentally to be Kexp ∼ 0.65 ± 0.1 in the case of the deuterium decoration of both kinds of radiation-induced defects with low and high de-trapping energies for deuterium. We introduced the theoretical estimation for coefficient of similarity between neutron- and self-ion-irradiations, which is a fraction of common area under the curves of two overlapping damage energy spectra of primary knock-on atom (PKA) produced in tungsten by these two types of irradiation. In other words, Ksim is a part of displaced atoms produced in the similar conditions under two different types of irradiation. The theoretical values of Ksim = 0.34 and Ksim = 0.29 were obtained for tungsten target irradiated with 20 MeV self-ions in comparison to irradiation with neutrons in HFIR reactor (>0.1 MeV) and 14 MeV neutrons, respectively. The theoretical value of Ksim = 0.34 is about two times less than the experimental value of Kexp = 0.65. It means that high energy PKAs can play more important role in the production of similar damage structure by irradiation with self-ions and neutrons which is responsible for deuterium retention. The model assuming that all cascades with an energy higher than Tc = 150 keV split into identical sub-cascades gives the value of Ksim = 0.64 ± 0.01 for the coefficient of similarity between HFIR-neutron and 20 MeV self-ion irradiations that is in an agreement with experimental value of Kexp = 0.65 ± 0.1. Consequently, splitting of high-energy part of cascades might take

  18. Special nuclear material detection using pulsed neutron interrogation

    NASA Astrophysics Data System (ADS)

    Ruddy, Frank H.; Seidel, John G.; Flammang, Robert W.

    2007-04-01

    Pulsed neutron interrogation methods for detection of Special Nuclear Materials are being developed. Fast prompt neutrons from thermal neutron-induced fissions are detected in the time intervals following 100-μs neutron bursts from a pulsed D-T neutron generator operating at 1000 pulses per second. Silicon Carbide semiconductor neutron detectors are used to detect fission neutrons in the 30-840 μs time intervals following each 14-MeV D-T neutron pulse. Optimization of the neutron detectors has led to dramatic reduction of detector background and improvement of the signal-to-noise ratio for Special Nuclear Material detection. Detection of Special Nuclear Materials in the presence of lead, cadmium and plywood shielding has been demonstrated. Generally, the introduction of shielding leads to short thermal neutron die-away times of 100-200 μs or less. The pulsed neutron interrogation method developed allows detection of the neutron signal even when the die-away time is less than 100 μs.

  19. TEM observation of neutron-induced collision cascades in Bi-2212 single crystals

    NASA Astrophysics Data System (ADS)

    Aleksa, M.; Pongratz, P.; Eibl, O.; Sauerzopf, F. M.; Weber, H. W.; Li, T. W.; Kes, P. H.

    1998-03-01

    Several high-quality single crystals of the superconductor Bi 2Sr 2CaCu 2O 8 (Bi-2212) were exposed to three different neutron fluences in the central irradiation facility of the Triga Mark II reactor in Vienna in the form of pre-prepared and pre-characterized transmission electron microscopy (TEM) samples as well as in full crystalline form. We find that the radiation damage produced in Bi-2212 is very similar to that found previously in YBa 2Cu 3O 7- δ (Y-123) single crystals. The diameter of the amorphous cascade volume is 3.5 nm, the inwardly directed strain field is of approximately the same size, the density of cascades is 3.7×10 22 m -3 per 10 22 neutrons m -2 ( E>0.1 MeV) and their concentration scales linearly with neutron fluence. Based on these results and in view of the similar displacement cross-sections of the constituents of other high temperature superconductors, we conclude that the neutron-induced defects in high- Tc materials will generally have a diameter (including the strain field) of 5-7 nm.

  20. Dynamics of neutron-induced fission of 235U using four-dimensional Langevin equations

    NASA Astrophysics Data System (ADS)

    Pahlavani, M. R.; Mirfathi, S. M.

    2015-08-01

    Background: Langevin equations have been suggested as a key approach to the dynamical analysis of energy dissipation in excited nuclei, formed during heavy-ion fusion-fission reactions. Recently, a few researchers theoretically reported investigations of fission for light nuclei in a low excitation energy using the Langevin approach, without considering the contribution of pre- and post-scission particles and γ -ray emission. Purpose: We study the dynamical evolution of mass distribution of fission fragments, and neutron and γ -ray multiplicity for 236U as compound nuclei that are constructed after fusion of a neutron and 235U. Method: Energy dissipation of the compound nucleus through fission is calculated using the Langevin dynamical approach combined with a Monte Carlo method. Also the shape of the fissioning nucleus is restricted to "funny hills" parametrization. Results: Fission fragment mass distribution, neutron and γ -ray multiplicity, and the average kinetic energy of emitted neutrons and γ rays at a low excitation energy are calculated using a dynamical model, based on the four-dimensional Langevin equations. Conclusions: The theoretical results show reasonable agreement with experimental data and the proposed dynamical model can well explain the energy dissipation in low energy induced fission.

  1. PromptNuFlux: Prompt atmospheric neutrino flux calculator

    NASA Astrophysics Data System (ADS)

    Rottoli, Luca

    2015-11-01

    PromptNuFlux computes the prompt atmospheric neutrino flux E3Φ(GeV2/(cm2ssr)), including the total associated theory uncertainty, for a range of energies between E=103 GeV and E=107.5 GeV. Results are available for five different parametrizations of the input cosmic ray flux: BPL, H3P, H3A, H14a, H14b.

  2. Determination of fission neutron transmission through waste matrix material using neutron signal correlation from active assay of {sup 239}Pu

    SciTech Connect

    Hollas, C.L.; Arnone, G.; Brunson, G.; Coop, K.

    1996-09-01

    The accuracy of TRU (transuranic) waste assay using the differential die-away technique depends upon significant corrections to compensate for the effects of the matrix material in which the TRU waste is located. The authors have used a new instrument, the Combined Thermal/Epithermal Neutron (CTEN) instrument for the assay of TRU waste, to develop methods to improve the accuracy of these corrections. Neutrons from a pulsed 14-MeV neutron generator are moderated in the walls of the CTEN cavity and induce fission in the TRU material. The prompt neutrons from these fission events are detected in cadmium-wrapped {sup 3}He neutron detectors. They report new methods of data acquisition and analysis to extract correlation in the neutron signals resulting form fission during active interrogation. They use the correlation information in conjunction with the total number of neutrons to determine the fraction of fission neutrons transmitted through the matrix material into the {sup 3}He detectors. This determination allows them to cleanly separate the matrix effects into two processes: matrix modification upon the neutron interrogating flux and matrix modification upon the fraction of fission neutrons transmitted to the neutron detectors. This transmission information is also directly applied in a neutron multiplicity analysis in the passive assay of {sup 240}Pu.

  3. Measurement and analysis of activation induced in titanium with fusion peak neutrons

    NASA Astrophysics Data System (ADS)

    Klix, A.; Domula, A.; Forrest, R.; Zuber, K.

    2011-10-01

    The intense neutron flux densities in fusion reactor blankets produce activation in the blanket materials relevant to operational safety, decommissioning, etc. The aim of the present work is to check the European Activation System EASY-2007 for its capability to predict important gamma activities induced in titanium in a fusion neutron field. Many advanced low-activation materials for fusion applications contain titanium, most notably in the breeder material Li 2TiO 3. In the present work, a small sample of Ti was irradiated with the intense DT neutron generator of Technical University of Dresden. The gamma-radioactivity following irradiation was measured and nuclide activities were derived. For each of the measured gamma activities, the corresponding value was calculated with EASY, and calculation-to-experiment ratios ( C/ E) were determined. EASY predicted the induced gamma activities, isotopes of scandium, well with some overestimation for 47Sc. The results of this measurement together with available EXFOR and validated state-of-the-art activation libraries are discussed.

  4. Investigation of neutron-induced background in Magnetic-Recoil-Spectrometer CR-39 data using a DT neutron source and MCNP simulations

    NASA Astrophysics Data System (ADS)

    Milanese, Lucio M.; Frenje, Johan; Gatu Johnson, Maria; Lahmann, Brandon; Sio, Hong; Petrasso, Richard

    2015-11-01

    The Magnetic Recoil neutron Spectrometers (MRS) installed on the OMEGA laser facility and the National Ignition Facility (NIF) are routinely used to measure neutron yield, areal density and ion temperatures from DT implosions. The observed background in the lower-energy part of MRS spectra is significantly higher than expected from analysis of neutron-induced background data obtained in stand-alone CR-39 experiments at OMEGA. A possible explanation relates to the scattering of neutrons in the MRS housing vessel, which is not accounted for in current modeling. To test experimentally the impact of individual vessel components on the observed background, parts of the MRS housing have been mocked up and CR-39 data have been collected employing a DT neutron source. The experimental results are contrasted to MCNP simulations to improve our understanding of the mechanism behind the enhanced neutron background. The results will be used to correct measured spectra from OMEGA and the NIF to allow detailed analysis of lower energy data. This work was supported in part by NLUF, US DOE, and LLE.

  5. An ionization chamber with Frisch grids for studies of high-energy neutron-induced fission

    NASA Astrophysics Data System (ADS)

    Tutin, G. A.; Ryzhov, I. V.; Eismont, V. P.; Kireev, A. V.; Condé, H.; Elmgren, K.; Olsson, N.; Renberg, P.-U.

    2001-01-01

    A gridded ionization chamber for fission fragment detection is described. The chamber has been specially designed for use at the quasi-monoenergetic 7Li(p, n) neutron source at the The Svedberg Laboratory, Uppsala, Sweden. The detector permits measurements of fission fragment energy and emission angle for two targets with diameter of up to 10 cm. The time response of the chamber (⩽5 ns FWHM) is adequate to apply time-of-flight discrimination against background events induced by non-peak neutrons. Results of angular anisotropy measurements for the 232Th (n, f) and 238U(n, f) reactions in the 20-160 MeV energy range are given.

  6. Neutron-induced Fission Cross Section of 240242Pu up to En = 3 MeV

    NASA Astrophysics Data System (ADS)

    Salvador-Castiñeira, P.; Bryś, T.; Hambsch, F.-J.; Oberstedt, S.; Pretel, C.; Vidali, M.

    2014-05-01

    The neutron-induced fission cross sections of 240,242Pu have been measured at JRC-IRMM with incident neutron energy from 0.2 MeV up to 3 MeV. A Twin-Frisch Grid Ionization Chamber (TFGIC) has been used in a back-to-back geometry. The measurements have been performed using the secondary standards 237Np and 238U as a reference. The purity of the plutonium samples was 99.89% for 240Pu and 99.97% for 242Pu. The results obtained follow the ENDF/B-VII.1 evaluation for 240Pu, but some discrepancies are visible around E/n = 1 MeV for 242Pu. In addition, the spontaneous fission half-life has been measured for both isotopes.

  7. Nuclear Reaction Models Responsible for Simulation of Neutron-induced Soft Errors in Microelectronics

    SciTech Connect

    Watanabe, Y. Abe, S.

    2014-06-15

    Terrestrial neutron-induced soft errors in MOSFETs from a 65 nm down to a 25 nm design rule are analyzed by means of multi-scale Monte Carlo simulation using the PHITS-HyENEXSS code system. Nuclear reaction models implemented in PHITS code are validated by comparisons with experimental data. From the analysis of calculated soft error rates, it is clarified that secondary He and H ions provide a major impact on soft errors with decreasing critical charge. It is also found that the high energy component from 10 MeV up to several hundreds of MeV in secondary cosmic-ray neutrons has the most significant source of soft errors regardless of design rule.

  8. Neutron-Induced Fission Cross Sections Measurements at n_TOF

    SciTech Connect

    Audouin, L.; Tassan-Got, L.; Isaev, S.; Koehler, Paul Edward; Collaboration, n_TOF

    2008-01-01

    The neutron-induced fission cross sections of {sup 233}U, {sup 234}U, {sup 235}U, {sup 238}U, {sup 232}Th, {sup 237}Np, {sup 209}Bi, {sup nat}Pb have been measured at the n{_}TOF facility at CERN over 9 orders of magnitude in neutron energy using {sup 235}U as a reference. Parallel Plate Avalanche Counters were used to detect both fission fragments in coincidence, thus efficiently discriminating fissions from other reactions. Data benefit from the remarkable energy resolution of the n{_}TOF facility. They are found in overall good agreement with databases and previous measurements, but some clear discrepancies can be put in evidence. These data are the first full coverage of the high-energy region (up to 1 GeV).

  9. Angular distribution of products of ternary nuclear fission induced by cold polarized neutrons

    NASA Astrophysics Data System (ADS)

    Bunakov, V. E.; Kadmensky, S. G.; Kadmensky, S. S.

    2008-11-01

    Within quantum fission theory, angular distributions of products originating from the ternary fission of nuclei that is induced by polarized cold and thermal neutrons are investigated on the basis of a nonevaporative mechanism of third-particle emission and a consistent description of fission-channel coupling. It is shown that the inclusion of Coriolis interaction both in the region of the discrete and in the region of the continuous spectrum of states of the system undergoing fission leads to T-odd correlations in the aforementioned angular distributions. The properties of the TRI and ROT effects discovered recently, which are due to the interference between the fission amplitudes of neutron resonances, are explored. The results obtained here are compared with their counterparts from classic calculations based on the trajectory method.

  10. The rotation of scissioning nucleus considered trajectory calculations for ternary fission induced by cold polarized neutrons

    NASA Astrophysics Data System (ADS)

    Guseva, I.; Gusev, Yu.

    2009-10-01

    On the base of modified trajectory calculations the shift of angular distribution of α-particles accompanied the reaction 235U(n,f) induced by cold polarized neutrons is evaluated. It was supposed that angular distribution shift is caused by the rotation of nuclear system before scission. The orientation of a rotation motion is determined by the neutron spin polarization along and opposite to the beam direction. For the first time the estimation was done in the frame of trajectory calculations assuming the rotation motion of scissioning nucleus [1]. The result of the calculation is in a good agreement with experimental data of paper [2], where this new phenomenon was named as ROT-effect.

  11. Boron analysis for neutron capture therapy using particle-induced gamma-ray emission.

    PubMed

    Nakai, Kei; Yamamoto, Yohei; Okamoto, Emiko; Yamamoto, Tetsuya; Yoshida, Fumiyo; Matsumura, Akira; Yamada, Naoto; Kitamura, Akane; Koka, Masashi; Satoh, Takahiro

    2015-12-01

    The neutron source of BNCT is currently changing from reactor to accelerator, but peripheral facilities such as a dose-planning system and blood boron analysis have still not been established. To evaluate the potential application of particle-induced gamma-ray emission (PIGE) for boron measurement in clinical boron neutron capture therapy, boronophenylalanine dissolved within a cell culture medium was measured using PIGE. PIGE detected 18 μgB/mL f-BPA in the culture medium, and all measurements of any given sample were taken within 20 min. Two hours of f-BPA exposure was required to create a boron distribution image. However, even though boron remained in the cells, the boron on the cell membrane could not be distinguished from the boron in the cytoplasm. PMID:26242558

  12. Semiclassical description of TRI asymmetry in ternary fission induced by cold polarized neutrons

    SciTech Connect

    Bunakov, V. E.; Kadmensky, S. G.

    2011-11-15

    The possibility of semiclassically describing T-even TRI-type asymmetry in ternary fission induced by polarized neutrons is considered on the basis of employing Coriolis interaction that takes into account the coupling of a light charged particle to the collective rotation of a polarized fissile nucleus. It is shown that allowance for this interaction makes it possible to explain qualitatively the magnitudes of two asymmetry effects observed in light-charge-particle emission both within the semiclassical and within the quantum-mechanical approach. The difference in the relative magnitudes and signs of the effects between different target nuclei is associated with the interference contributions to the cross section from neighboring neutron resonances and therefore cannot be explained within the semiclassical approach.

  13. Angular distribution of products of ternary nuclear fission induced by cold polarized neutrons

    SciTech Connect

    Bunakov, V. E. Kadmensky, S. G. Kadmensky, S. S.

    2008-11-15

    Within quantum fission theory, angular distributions of products originating from the ternary fission of nuclei that is induced by polarized cold and thermal neutrons are investigated on the basis of a non-evaporative mechanism of third-particle emission and a consistent description of fission-channel coupling. It is shown that the inclusion of Coriolis interaction both in the region of the discrete and in the region of the continuous spectrum of states of the system undergoing fission leads to T-odd correlations in the aforementioned angular distributions. The properties of the TRI and ROT effects discovered recently, which are due to the interference between the fission amplitudes of neutron resonances, are explored. The results obtained here are compared with their counterparts from classic calculations based on the trajectory method.

  14. Chromosome aberrations induced in human lymphocytes by D-T neutrons

    SciTech Connect

    Lloyd, D.C.; Edwards, A.A.; Prosser, J.S.; Bolton, D.; Sherwin, A.G.

    1984-06-01

    Unstable chromosome aberrations induced by in vitro irradiation with D-T neutrons have been analyzed in human blood lymphocytes. With respect to 250 kVp X rays a maximum limiting RBE at low doses of 4.1 was obtained for dicentric aberrations. Using aberrations as markers in mixed cultures of irradiated and unirradiated cells permits an assessment of interphase death plus mitotic delay. The low-dose RBE for this effect is 2.5. Assuming all unstable aberrations observed at metaphase would lead to cell death by nondisjunction allows an assessment of mitotic death. The low-dose RBE for this effect is 4.5. The data are compared with similar work obtained earlier with /sup 242/Cm ..cap alpha.. particles. The application of the present work to cytogenetic assessment of dose after accidental exposure to D-T neutrons is discussed.

  15. Neutron dosimetry

    DOEpatents

    Quinby, Thomas C.

    1976-07-27

    A method of measuring neutron radiation within a nuclear reactor is provided. A sintered oxide wire is disposed within the reactor and exposed to neutron radiation. The induced radioactivity is measured to provide an indication of the neutron energy and flux within the reactor.

  16. Radioactive ion beams produced by neutron-induced fission at ISOLDE

    NASA Astrophysics Data System (ADS)

    Isolde Collaboration; Catherall, R.; Lettry, J.; Gilardoni, S.; Köster, U.

    2003-05-01

    The production rates of neutron-rich fission products for the next-generation radioactive beam facility EURISOL [EU-RTD Project EURISOL (HPRI-CT-1999-50001)] are mainly limited by the maximum amount of power deposited by protons in the target. An alternative approach is to use neutron beams to induce fission in actinide targets. This has the advantage of reducing: the energy deposited by the proton beam in the target; contamination from neutron-deficient isobars that would be produced by spallation; and mechanical stress on the target. At ISOLDE CERN [E. Kugler, Hyperfine Interact. 129 (2000) 23], tests have been made on standard ISOLDE actinide targets using fast-neutron bunches produced by bombarding thick, high-/Z metal converters with 1 and 1.4 GeV proton pulses. This paper reviews the first applications of converters used at ISOLDE. It highlights the different geometries and the techniques used to compare fission yields produced by the proton beam directly on the target with neutron-induced fission. Results from the six targets already tested, namely UC2/graphite and ThO2 targets with tungsten and tantalum converters, are presented. To gain further knowledge for the design of a dedicated target as required by the TARGISOL project [EU-RTD Project TARGISOL (HPRI-CT-2001-50033)], the results are compared to simulations, using the MARS [N.V. Mokhov, S.I. Striganov, A. Van Ginneken, S.G. Mashnik, A.J. Sierk, J. Ranft, MARS code developments, in: 4th Workshop on Simulating Accelerator Radiation Environments, SARE-4, Knoxville, USA, 14-15.9.1998, FERMILAB-PUB-98-379, nucl-th/9812038; N.V. Mokhov, The Mars Code System User's Guide, Fermilab-FN-628, 1995; N.V. Mokhov, MARS Code Developments, Benchmarking and Applications, Fermilab-Conf-00-066, 2000; O.E. Krivosheev, N.V. Mokhov, A New MARS and its Applications, Fermilab-Conf-98/43, 1998] code interfaced with MCNP [J.S. Hendrics, MCNP4C LANL Memo X-5; JSH-2000-3; J.F. Briemesteir (Ed.), MCNP - A General Montecarlo N

  17. RECENT APPLICATIONS OF THE GREENSPAN AND TSCHIEGG DATA ON NEUTRON INDUCED CAVITATION THRESHOLDS

    SciTech Connect

    West, Colin D

    2007-03-01

    In 1967 Greenspan and Tschiegg published a paper on radiation induced acoustic cavitation. They researched the thresholds for cavitation induced in various liquids by fast neutrons, {alpha}-decay recoils and fission fragments. It turns out that these data can be used to verify predictions of a more recent theory of radiation induced cavitation nucleation. In 1979, in a report to their sponsor (The Office of Naval Research) they published new details of their results on neutron induced cavitation thresholds, including tables of the thresholds at different temperatures for various liquids. They were also some fission fragment results, but none of the {alpha}-decay recoil data. By that time Greenspan had evidently retired while I had left the field of cavitation research and did not know of the existence of their report [which also contains the only published record of some cavitation threshold measurements made by West and Howlett at Harwell, England]. Later still, in 1982, Greenspan and Tschiegg published the graphical data--but not the tables--in a more easily accessible form. In the late 1990s I revisited the problem of calculating radiation induced cavitation thresholds. There was interest in this because the Spallation Neutron Source (SNS) project, then just beginning, planned to use a liquid mercury target to produce intense bursts of neutrons when irradiated by a pulsed, high energy proton beam. It was known that the pressure waves produced by local heating when the proton pulse struck the target could, upon reflection at the walls of the mercury container, give rise to very high, although brief, negative pressure waves in the mercury. There was concern that cavitation might result and, if it did, might lead to undesirable effects. With the encouragement of the SNS target team this author managed further to develop an earlier method of calculating the threshold for such cavitation, and the SNS project kindly provided funding to publish the work in two ORNL

  18. Measurement of residual 152Eu activity induced by atomic bomb neutrons in Nagasaki and the contribution of environmental neutrons to this activity.

    PubMed

    Shizuma, Kiyoshi; Endo, Satoru; Hoshi, Masaharu; Takada, Jun; Ishikawa, Masayori; Iwatani, Kazuo; Hasai, Hiromi; Oka, Takamitsu; Fujita, Shoichiro; Watanabe, Tadaaki; Yamashita, Tomoaki; Imanaka, Tetsuji

    2003-06-01

    Residual 152Eu activities induced by neutrons from the Nagasaki atomic bomb were measured for nine mineral samples located up to 1,061 m in the slant range and one control sample at 2,850 m from the hypocenter. A chemical separation to prepare europium-enriched samples was performed for all samples, and gamma ray measurements were carried out with a low background well-type germanium detector. In this paper, the measured specific activities of 152Eu are compared with activation calculations based on the DS86 neutron fluence and the 93Rev one. The calculated-to-measured ratios are also compared with those of 60Co and 36Cl. The present results indicate that the measurements agree to the calculation within a factor of three as observed in the nuclear tests at Nevada. The activation level of environmental neutrons and the detection limit for 152Eu are also discussed. PMID:13678342

  19. Effects of Neutron Emission on Fragment Mass and Kinetic Energy Distribution from Thermal Neutron-Induced Fission of {sup 235}U

    SciTech Connect

    Montoya, M.; Rojas, J.; Saetone, E.

    2007-10-26

    The mass and kinetic energy distribution of nuclear fragments from thermal neutron-induced fission of {sup 235}U(n{sub th},f) have been studied using a Monte-Carlo simulation. Besides reproducing the pronounced broadening in the standard deviation of the kinetic energy at the final fragment mass number around m = 109, our simulation also produces a second broadening around m = 125. These results are in good agreement with the experimental data obtained by Belhafaf et al. and other results on yield of mass. We conclude that the obtained results are a consequence of the characteristics of the neutron emission, the sharp variation in the primary fragment kinetic energy and mass yield curves. We show that because neutron emission is hazardous to make any conclusion on primary quantities distribution of fragments from experimental results on final quantities distributions.

  20. Time dependent measurements of induced fission for SNM interrogation

    NASA Astrophysics Data System (ADS)

    Beck, A.; Israelashvili, I.; Wengrowicz, U.; Caspi, E. N.; Yaar, I.; Osovizki, A.; Ocherashvili, A.; Rennhofer, H.; Pedersen, B.; Crochemore, J.-M.; Roesgen, E.

    2013-08-01

    Gammas from induced fissions were measured and separated into prompt and delayed particles. To this end, a dedicated detector was realized, based on a plastic scintillator, a wavelength shifter fiber and a silicon photomultiplier (SiPM). Results are presented from the interrogation of Special Nuclear Materials (SNM), employing a pulsed neutron generator in the PUNITA graphite moderator incorporating the above detector assembly. The detector response is presented, as well as the sensitivities for prompt and delayed processes within the same experimental setup.

  1. Continuous versus pulse neutron induced gamma spectroscopy for soil carbon analysis.

    PubMed

    Kavetskiy, A; Yakubova, G; Torbert, H A; Prior, S A

    2015-02-01

    Neutron induced gamma spectra analysis (NGA) provides a means of measuring carbon in large soil volumes without destructive sampling. Calibration of the NGA system must account for system background and the interference of other nuclei on the carbon peak at 4.43 MeV. Accounting for these factors produced measurements in agreement with theoretical considerations. The continuous NGA mode was twice as fast and just as accurate as the pulse mode, thus this mode was preferable for routine soil carbon analysis. PMID:25497322

  2. Feeding of isomers of stable Rh, Ag, Ir and Au isotopes in fast-neutron-induced reactions

    NASA Astrophysics Data System (ADS)

    Fotiades, N.; Devlin, M.; Nelson, R. O.; Carroll, J. J.

    2016-03-01

    The GEANIE spectrometer, comprised of 20 high-purity Ge detectors coupled to the broad-spectrum pulsed neutron beam of the Los Alamos Neutron Science Center's (LANSCE) WNR facility, has been used to determine partial γ-ray cross sections in (n , xn) fast-neutron-induced reactions. In (n ,n') reactions on stable Ir and Au isotopes the γ-ray feeding, as established with GEANIE, for the isomers relative to the feeding of the corresponding ground states increases with increasing neutron energy up to the neutron energy where the (n , 2 n) reaction channel opens and then decreases. The behavior in mass A = 100 region of the γ-ray feeding of isomers and ground states was also studied with GEANIE in fast-neutron-induced reactions on stable Rh and Ag isotopes. The feeding of the isomers was found to be very similar in the corresponding reaction channels and it was compared to the feeding determined for the ground states. The opening of higher-neutron-emitting reaction channels remove angular momentum from the compound system and reduce the population of higher-spin isomers relative to the feeding of lower-spin ground states in all cases studied.

  3. Methods and procedures for evaluation of neutron-induced activation cross sections

    SciTech Connect

    Gardner, M.A.

    1981-09-01

    One cannot expect measurements alone to supply all of the neutron-induced activation cross-section data required by the fission reactor, fusion reactor, and nuclear weapons development communities, given the wide ranges of incident neutron energies, the great variety of possible reaction types leading to activation, and targets both stable and unstable. Therefore, the evaluator must look to nuclear model calculations and systematics to aid in fulfilling these cross-section data needs. This review presents some of the recent developments and improvements in the prediction of neutron activation cross sections, with specific emphasis on the use of empirical and semiempirical methods. Since such systematics require much less nuclear informaion as input and much less computational time than do the multistep Hauser-Feshbach codes, they can often provide certain cross-section data at a sufficient level of accuracy within a minimum amount of time. The cross-section information that these systematics can and cannot provide and those cases in which they can be used most reliably are discussed.

  4. Reliability Design for Neutron Induced Single-Event Burnout of IGBT

    NASA Astrophysics Data System (ADS)

    Shoji, Tomoyuki; Nishida, Shuichi; Ohnishi, Toyokazu; Fujikawa, Touma; Nose, Noboru; Hamada, Kimimori; Ishiko, Masayasu

    Single-event burnout (SEB) caused by cosmic ray neutrons leads to catastrophic failures in insulated gate bipolar transistors (IGBTs). It was found experimentally that the incident neutron induced SEB failure rate increases as a function of the applied collector voltage. Moreover, the failure rate increased sharply with an increase in the applied collector voltage when the voltage exceeded a certain threshold value (SEB cutoff voltage). In this paper, transient device simulation results indicate that impact ionization at the n-drift/n+ buffer boundary is a crucially important factor in the turning-on of the parasitic pnp transistor, and eventually latch-up of the parasitic thyristor causes SEB. In addition, the device parameter dependency of the SEB cutoff voltage was analytically derived from the latch-up condition of the parasitic thyristor. As a result, it was confirmed that reducing the current gain of the parasitic transistor, such as by increasing the n-drift region thickness d was effective in increasing the SEB cutoff voltage. Furthermore, `white' neutron-irradiation experiments demonstrated that suppressing the inherent parasitic thyristor action leads to an improvement of the SEB cutoff voltage. It was confirmed that current gain optimization of the parasitic transistor is a crucial factor for establishing highly reliable design against chance failures.

  5. Study of Neutron-Induced Fission Cross Sections of U, Am, and Cm at n{sub T}OF

    SciTech Connect

    Milazzo, P. M.; Abbondanno, U.; Belloni, F.; Fujii, K.; Aerts, G.; Andriamonje, S.; Berthoumieux, E.; Dridi, W.; Ferrant, L.; Gunsing, F.; Pancin, J.; Perrot, L.; Plukis, A.; Stephan, C.; Tassan-Got, L.; Alvarez-Velarde, F.; Cano-Ott, D.

    2010-08-04

    Neutron induced fission cross sections of several isotopes have been measured at the CERN n{sub T}OF spallation neutron facility. Between them some measurements involve isotopes ({sup 233}U, {sup 241}Am, {sup 243}Am, {sup 245}Cm) relevant for applications to nuclear technologies. The n{sub T}OF facility delivers neutrons with high instantaneous flux and in a wide energy range, from thermal up to 250 MeV. The experimental apparatus consists of an ionization chamber that discriminates fission fragments and {alpha} particles coming from natural radioactivity of the samples. All the measurements were performed referring to the standard cross section of {sup 235}U.

  6. Nuclear interaction of Smac/DIABLO with Survivin at G2/M arrest prompts docetaxel-induced apoptosis in DU145 prostate cancer cells

    SciTech Connect

    Kim, Ji Young; Chung, Jin-Yong; Lee, Seung Gee; Kim, Yoon-Jae; Park, Ji-Eun; Yoo, Ki Soo; Yoo, Young Hyun; Park, Young Chul; Kim, Byeong Gee; Kim, Jong-Min . E-mail: jmkim7@dau.ac.kr

    2006-12-01

    Smac/DIABLO is released by mitochondria in response to apoptotic stimuli and is thought to antagonize the function of inhibitors of apoptosis proteins. Recently, it has been shown that, like XIAP, Survivin can potentially interact with Smac/DIABLO. However, the precise mechanisms and cellular location of their action have not been determined. We report for the first time that Smac/DIABLO translocates to the nucleus and is colocalized with Survivin at mitotic spindles during apoptosis resulting from G2/M arrest due to docetaxel treatment of DU145 prostate cancer cells. Our data demonstrate that the nuclear interaction of Smac/DIABLO with Survivin is an important step for suppressing the anti-apoptotic function of Survivin in Doc-induced apoptosis. This suggests that the balance between cellular Smac/DIABLO and Survivin levels could be critical for cellular destiny in taxane-treated cancer cells.

  7. Influence of secondary neutrons induced by proton radiotherapy for cancer patients with implantable cardioverter defibrillators

    PubMed Central

    2012-01-01

    Background Although proton radiotherapy is a promising new approach for cancer patients, functional interference is a concern for patients with implantable cardioverter defibrillators (ICDs). The purpose of this study was to clarify the influence of secondary neutrons induced by proton radiotherapy on ICDs. Methods The experimental set-up simulated proton radiotherapy for a patient with an ICD. Four new ICDs were placed 0.3 cm laterally and 3 cm distally outside the radiation field in order to evaluate the influence of secondary neutrons. The cumulative in-field radiation dose was 107 Gy over 10 sessions of irradiation with a dose rate of 2 Gy/min and a field size of 10 × 10 cm2. After each radiation fraction, interference with the ICD by the therapy was analyzed by an ICD programmer. The dose distributions of secondary neutrons were estimated by Monte-Carlo simulation. Results The frequency of the power-on reset, the most serious soft error where the programmed pacing mode changes temporarily to a safety back-up mode, was 1 per approximately 50 Gy. The total number of soft errors logged in all devices was 29, which was a rate of 1 soft error per approximately 15 Gy. No permanent device malfunctions were detected. The calculated dose of secondary neutrons per 1 Gy proton dose in the phantom was approximately 1.3-8.9 mSv/Gy. Conclusions With the present experimental settings, the probability was approximately 1 power-on reset per 50 Gy, which was below the dose level (60-80 Gy) generally used in proton radiotherapy. Further quantitative analysis in various settings is needed to establish guidelines regarding proton radiotherapy for cancer patients with ICDs. PMID:22284700

  8. Prompt proton decay in the vicinity of {sup 56}Ni

    SciTech Connect

    Johansson, E. K.; Rudolph, D.; Andersson, L-L.; Fahlander, C.; Rietz, R. du; Torres, D. A.; Carpenter, M. P.; Seweryniak, D.; Zhu, S.; Charity, R. J.; Chiara, C. J.; Hoel, C.; Pechenaya, O. L.; Reviol, W.; Sarantites, D. G.; Sobotka, L. G.; Ekman, J.

    2007-11-30

    A new decay mode, the so called prompt proton decay, was discovered in 1998. It has since proven to be an important decay mechanism for several neutron deficient nuclei in the A{approx}60 region. To measure with high accuracy the energies and angular distributions of these protons, a state-of-the-art charged particle detector--LuWuSiA--was developed. It was first utilized during a fusion-evaporation reaction experiment performed at Argonne National Laboratory, U.S.A. In this contribution, the characteristics of the prompt proton decay are discussed along with the special features of LuWuSiA as well as a revisit to the prompt proton decay in {sup 58}Cu.

  9. Total prompt γ-ray emission in fission of U235, Pu239,241, and Cf252

    NASA Astrophysics Data System (ADS)

    Chyzh, A.; Wu, C. Y.; Kwan, E.; Henderson, R. A.; Bredeweg, T. A.; Haight, R. C.; Hayes-Sterbenz, A. C.; Lee, H. Y.; O'Donnell, J. M.; Ullmann, J. L.

    2014-07-01

    The total prompt γ-ray energy distributions for the neutron-induced fission of U235 and Pu239,241 in the neutron energy range of 0.025 eV - 100 keV and the spontaneous fission of Cf252 were measured using the Detector for Advanced Neutron Capture Experiments (DANCE) in coincidence with the detection of fission fragments by a parallel-plate avalanche counter. DANCE is a highly segmented, highly efficient 4π γ-ray calorimeter. Corrections were made to the measured distribution by unfolding the two-dimension spectrum of total γ-ray energy vs multiplicity using a simulated DANCE response matrix generated with a geometrical model of the detector arrays and validated with the γ-ray calibration sources. The mean values of the total prompt γ-ray energy, determined from the unfolded distributions, are ˜20% higher than those of early measurements for all the fissile nuclei studied. The implication for the γ heating in nuclear reactors is discussed.

  10. Neutron irradiation induced microstructural changes in NBG-18 and IG-110 nuclear graphites

    SciTech Connect

    Karthik, Chinnathambi; Kane, Joshua; Butt, Darryl P.; Windes, William E.; Ubic, Rick

    2015-05-01

    This paper reports the neutron-irradiation-induced effects on the microstructure of NBG-18 and IG-110 nuclear graphites. The high-temperature neutron irradiation at two different irradiation conditions was carried out at the Advanced Test Reactor National User Facility at the Idaho National Laboratory. NBG-18 samples were irradiated to 1.54 dpa and 6.78 dpa at 430 °C and 678 °C respectively. IG-110 samples were irradiated to 1.91 dpa and 6.70 dpa at 451 °C and 674 °C respectively. Bright-field transmission electron microscopy imaging was used to study the changes in different microstructural components such as filler particles, microcracks, binder and quinoline-insoluble (QI) particles. Significant changes have been observed in samples irradiated to about 6.7 dpa. The closing of pre-existing microcracks was observed in both the filler and the binder phases. The binder phase exhibited substantial densification with near complete elimination of the microcracks. The QI particles embedded in the binder phase exhibited a complete microstructural transformation from rosettes to highly crystalline solid spheres. The lattice images indicate the formation of edge dislocations as well as extended line defects bridging the adjacent basal planes. The positive climb of these dislocations has been identified as the main contributor to the irradiation-induced swelling of the graphite lattice.

  11. Neutron-induced autoradiography used in the investigation of modern pigments in paintings of known composition

    SciTech Connect

    Aderhold, H.C.; Taft, W.S.

    1992-07-01

    Neutron-Induced Autoradiography is an effective analytical technique for mapping the location of a number of specified pigments in paintings. Most paintings which have been examined through neutron-induced autoradiography to date were painted prior to the introduction of the most common of modern pigments. By understanding die nuclear properties of these pigments, as revealed by this technique, a more informed analysis of modem paintings may result This investigation is part of an ongoing program to develop case studies for presentation to an undergraduate class at Cornell University, 'Art, Isotopes and Analysis'. We have found that this technique is a graphic and effective method of presenting nuclear reactions and radioactivity to non-specialists. Sample paintings are produced using pigments of known composition. A sequence of discreet layers, each a separate image, is documented in order to establish a reference for accurately interpreting the autoradiographs. The painting is then activated in the Cornell TRIGA reactor and a series of autoradiographs produced Gamma spectra taken before and after each film exposure gives us detailed information on which radioisotopes (and therefore, which pigments), are active. (author)

  12. Detection of special nuclear material from delayed neutron emission induced by a dual-particle monoenergetic source

    NASA Astrophysics Data System (ADS)

    Mayer, M.; Nattress, J.; Jovanovic, I.

    2016-06-01

    Detection of unique signatures of special nuclear materials is critical for their interdiction in a variety of nuclear security and nonproliferation scenarios. We report on the observation of delayed neutrons from fission of uranium induced in dual-particle active interrogation based on the 11B(d,n γ)12C nuclear reaction. Majority of the fissions are attributed to fast fission induced by the incident quasi-monoenergetic neutrons. A Li-doped glass-polymer composite scintillation neutron detector, which displays excellent neutron/γ discrimination at low energies, was used in the measurements, along with a recoil-based liquid scintillation detector. Time-dependent buildup and decay of delayed neutron emission from 238U were measured between the interrogating beam pulses and after the interrogating beam was turned off, respectively. Characteristic buildup and decay time profiles were compared to the common parametrization into six delayed neutron groups, finding a good agreement between the measurement and nuclear data. This method is promising for detecting fissile and fissionable materials in cargo scanning applications and can be readily integrated with transmission radiography using low-energy nuclear reaction sources.

  13. Initial observations of cavitation-induced erosion of liquid metal spallation target vessels at the Spallation Neutron Source

    SciTech Connect

    McClintock, David A; Riemer, Bernie; Ferguson, Phillip D; Carroll, Adam J; Dayton, Michael J

    2012-01-01

    During operation of the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory the mechanical properties of the AISI 316L target module are altered by high-energy neutron and proton radiation. The interior surfaces of the target vessel are also damaged by cavitation-induced erosion, which results from repetitive rapid heating of the liquid mercury by high-energy proton beam pulses. Until recently no observations of cavitation-induced erosion were possible for conditions prototypical to the SNS. Post irradiation examination (PIE) of the first and second operational SNS targets was performed to gain insight into the radiation-induced changes in mechanical properties of the 316L target material and the extent of cavitation-induced erosion to the target vessel inner surfaces. Observations of cavitation-induced erosion of the first and second operational SNS target modules are presented here, including images of the target vessel interiors and specimens removed from the target beam-entrance regions.

  14. Extensions of the burst generation rate method for wider application to proton/neutron-induced single event effects

    SciTech Connect

    Normand, E.

    1998-12-01

    The Burst Generation Rate (BGR) method, originally developed to calculate single event upset (SEU) rates in microelectronics due to neutrons and protons, has been extended for wider application, allowing cross sections for both SEU and single event latchup (SEL) to be calculated, and comparisons to be made with measured data. The method uses the Weibull fit to accurately represent the behavior of the heavy ion SEU cross section. Proton SEU cross sections in RAMs, microprocessors and FPGAs are calculated, with agreement generally to within a factor of 2--3, and similar results are obtained for neutron cross sections for both cosmic ray and fission spectra. The BGR method is also modified to calculate cross sections for proton/neutron induced SEL. Agreement is generally good for SEL for most devices, but there are also limitations, since some very modern devices are shown to have unusually high susceptibility to SEL by protons/neutrons.

  15. Rotation of Nuclei as Observed in Ternary Fission of the Reaction 235U(nth,f) Induced by Polarized Neutron

    NASA Astrophysics Data System (ADS)

    Gönnenwein, F.; Gagarski, A.; Guseva, I.; Petrov, G.; Sokolov, V.; Zavarukhkina, T.; Mutterer, M.; Nesvizhevski, V.; Bunakov, V.; Kadmensky, S.

    2007-05-01

    Ternary fission of the standard reaction 235U(nth,f) induced by cold polarized neutrons has been investigated. Fission fragments and light charged particles were recorded in coincidence. Following cold neutron capture the compound nucleus 236U* has spin 3- or 4-. At the saddle point of the fissioning 236U* nucleus these states are collective. They are expected to retain a sizable collectivity down to the scission point. In fact, a collective rotation has been sensed by the shift in the angular distribution of the light charged particles which depends on the orientation of neutron polarization. Direct observation of the rotation of 236U* excited in a cold neutron reaction is reported here for the first time. It is proposed to call the new phenomenon the "ROT-effect".

  16. Thermal Neutron Imaging in an Active Interrogation Environment

    SciTech Connect

    Vanier, Peter E.; Forman, Leon; Norman, Daren R.

    2009-03-10

    We have developed a thermal-neutron coded-aperture imager that reveals the locations of hydrogenous materials from which thermal neutrons are being emitted. This imaging detector can be combined with an accelerator to form an active interrogation system in which fast neutrons are produced in a heavy metal target by means of excitation by high energy photons. The photo-induced neutrons can be either prompt or delayed, depending on whether neutron-emitting fission products are generated. Provided that there are hydrogenous materials close to the target, some of the photo-induced neutrons slow down and emerge from the surface at thermal energies. These neutrons can be used to create images that show the location and shape of the thermalizing materials. Analysis of the temporal response of the neutron flux provides information about delayed neutrons from induced fission if there are fissionable materials in the target. The combination of imaging and time-of-flight discrimination helps to improve the signal-to-background ratio. It is also possible to interrogate the target with neutrons, for example using a D-T generator. In this case, an image can be obtained from hydrogenous material in a target without the presence of heavy metal. In addition, if fissionable material is present in the target, probing with fast neutrons can stimulate delayed neutrons from fission, and the imager can detect and locate the object of interest, using appropriate time gating. Operation of this sensitive detection equipment in the vicinity of an accelerator presents a number of challenges, because the accelerator emits electromagnetic interference as well as stray ionizing radiation, which can mask the signals of interest.

  17. Neutron induced fission of U isotopes up to 100 MeV

    SciTech Connect

    Lestone, J.P.; Gavron, A.

    1993-10-01

    We have developed a statistical model description of the neutron induced fission of U isotopes using densities of intrinsic states and spin cut off parameters obtained directly from appropriate Nilsson model single particle levels. The first chance fission cross sections are well reproduced when the rotational contributions to the nuclear level densities are taken into account. In order to fit the U(n,f) cross sections above the threshold of second chance fission, we need to: (1) assume that the triaxial level density enhancement is washed out at an excitation energy of {approximately}7 MeV above the triaxial barriers with a width of {approximately}1 MeV, implying a {gamma} deformation for the first barriers of 10{degree} < {gamma} < 20{degree}; and (2) include pre-equilibrium particle emission in the calculations. Above an incoming neutron kinetic energy of {approximately}17 MeV our statistical model U(n,f) cross sections increasingly overestimate the experimental data when so called ``good`` optical model potentials are used to calculate the compound nucleus formation cross sections. This is not surprising since at these high energies little data exists on the scattering of neutrons to help guide the choice of optical model parameters. A satisfactory reproduction of all the available U(n,f) cross sections above 17 MeV is obtained by a simple scaling of our calculated compound nucleus formation cross sections. This scaling factor falls from 1.0 at 17 MeV to 0.82 at 100 MeV.

  18. 196Pt(n,xn yp γ) reactions using spallation neutrons from En=1 to 250 MeV

    NASA Astrophysics Data System (ADS)

    Tavukcu, E.; Bernstein, L. A.; Hauschild, K.; Becker, J. A.; Garrett, P. E.; McGrath, C. A.; McNabb, D. P.; Younes, W.; Chadwick, M. B.; Nelson, R. O.; Johns, G. D.; Mitchell, G. E.

    2001-11-01

    Neutron-induced reactions on 196Pt were studied over the neutron energy range from 1 to 250 MeV. A ``white'' neutron beam was provided by the spallation neutron source of the Weapons Neutron Research facility at the Los Alamos Neutron Science Center. The prompt reaction γ rays were measured with the large-scale Compton-suppressed Ge spectrometer GEANIE. The incident neutron energy was determined by the time-of-flight technique. Excitation functions for γ-ray transitions in 184,186,188,190-196Pt and 189,191,193Ir isotopes are compared with enhanced Hauser-Feshbach reaction modeling, as implemented in the reaction code GNASH. Overall, the model predictions agree well with the measured γ-ray yields. Discrepancies appear, however, due to inadequate discrete-level information in the calculations describing the preequilibrium process.

  19. Revised Production Rates for Na-22 and Mn-54 in Meteorites Using Cross Sections Measured for Neutron-induced Reactions

    NASA Technical Reports Server (NTRS)

    Sisterson, J. M.; Kim, K. J.; Reedy, R. C.

    2004-01-01

    The interactions of galactic cosmic rays (GCR) with extraterrestrial bodies produce small amounts of radionuclides and stable isotopes. The production rates of many relatively short-lived radionuclides, including 2.6-year Na-22 and 312-day Mn-54, have been measured in several meteorites collected very soon after they fell. Theoretical models used to calculate production rates for comparison with the measured values rely on input data containing good cross section measurements for all relevant reactions. Most GCR particles are protons, but secondary neutrons make most cosmogenic nuclides. Calculated production rates using only cross sections for proton-induced reactions do not agree well with measurements. One possible explanation is that the contribution to the production rate from reactions initiated by secondary neutrons produced in primary GCR interactions should be included explicitly. This, however, is difficult to do because so few of the relevant cross sections for neutron-induced reactions have been measured.

  20. Neutrons scattering studies in the actinide region. Progress report, August 1, 1991--July 31, 1992

    SciTech Connect

    Kegel, G.H.R.; Egan, J.J.

    1992-09-01

    During the report period were investigated the following areas: prompt fission neutron energy spectra measurements; neutron elastic and inelastic scattering from {sup 239}Pu; neutron scattering in {sup 181}Ta and {sup 197}Au; response of a {sup 235}U fission chamber near reaction thresholds; two-parameter data acquisition system; ``black`` neutron detector; investigation of neutron-induced defects in silicon dioxide; and multiple scattering corrections. Four Ph.D. dissertations and one M.S. thesis were completed during the report period. Publications consisted of three journal articles, four conference papers in proceedings, and eleven abstracts of presentations at scientific meetings. There are currently four Ph.D. and one M.S. candidates working on dissertations directly associated with the project. In addition, three other Ph.D. candidates are working on dissertations involving other aspects of neutron physics in this laboratory.

  1. Decay radioactivity induced in plasma-facing materials by deutrium-tritium neutrons

    SciTech Connect

    Kumar, A.; Abdou, M.A.; Youssef, M.Z.; Ikeda, Y.; Konno, C.; Kosako, K.; Oyama, Y.; Nakamura, T.; Maekawa, H.

    1995-08-01

    Deuterium-tritium (D-T) neutron-induced radioactivity constitutes one of the foremost issues in fusion reactor design. Designers have been using radioactivity codes and associated nuclear data libraries for nucleonic designs of fusion reactors. However, in the past, there was hardly any experimental validation of these codes/libraries. An elaborate, experimental program was initiated in 1988 under a U.S. Department of Energy/Japan Atomic Energy Research Institute collaborative program to validate the radioactivity codes/libraries. As many as 14 neutron energy spectra were covered for a number of materials. The analyses of the isotopic activities of the irradiated materials using the activation cross-section libraries of four leading radioactivity codes, i.e., ACT4/THIDA-1, REAC-3. DKR-ICF; and RACC, have shown large discrepancies among the calculations on one hand and between the calculations and the measurements, on the other. Vanadium, Co, Ni, Zn, Zr, Mo, In, Sn, and W each count the largest number of discrepant isotopic activities. In addition to providing detailed results of the status of predictability of individual isotopic activities using the ACT4, REAC-3, DKR-ICF, and RACC activation cross-section libraries, safety factors cum quality factors characterizing each library are presented and discussed. The related issues of confidence level and associated uncertainty are also highlighted. 37 refs., 112 figs., 24 tabs.

  2. Neutron stars and millisecond pulsars from accretion-induced collapse in globular clusters

    NASA Technical Reports Server (NTRS)

    Bailyn, Charles D.; Grindlay, Jonathan E.

    1990-01-01

    This paper examines the limits on the number of millisecond pulsars which could be formed in globular clusters by the generally accepted scenario (in which a neutron star is created by the supernova of an initially massive star and subsequently captures a companion to form a low-mass X-ray binary which eventually becomes a millisecond pulsar). It is found that, while the number of observed low-mass X-ray binaries can be adequately explained in this way, the reasonable assumption that the pulsar luminosity function in clusters extends below the current observational limits down to the luminosity of the faintest millisecond pulsars in the field suggests a cluster population of millisecond pulsars which is substantially larger than the standard model can produce. Alleviating this problem by postulating much shorter lifetimes for the X-ray binaries requires massive star populations sufficiently large that the mass loss resulting from their evolution would be likely to unbind the cluster. It is argued that neutron star formation in globular clusters by accretion-induced collapse of white dwarfs may resolve the discrepancy in birthrates.

  3. Neutron Induced Backgrounds In the MIXE X-Ray Detector at Balloon Altitudes

    NASA Technical Reports Server (NTRS)

    Armstrong, T. W.; Colborn, B. L.; Dietz, K. L.; Ramsey, B. D.

    1997-01-01

    The MIXE detector developed at NASA/MSFC is designed for x-ray astronomy and consists of a multiwire proportional counter sensitive to photons less than 150 keV. The detector has been flown on several balloon flights with higher than expected background levels observed. Previous predictions of the detector background due to atmospheric gamma-ray and cosmic diffuse sources were much less (factor of 3) than flight background measurements. The work reported here was undertaken to determine if the additional contribution from gamma-rays generated by albedo and cosmic-ray induced neutrons in the detector and payload assembly could account for the background levels observed. Monte Carlo nuclear interaction and radiation transport simulations were made for the ambient cosmic-ray environment corresponding to a previous MEE balloon flight at 3 g/cm(exp 2) residual atmosphere and 42 N geomagnetic latitude. The omnidirectional albedo neutron spectrum and the GCR proton spectrum which were used as input to the calculations are shown. For the albedo angular distribution, the predicted up/down flux ratio of 2.5 was used together with the angular dependence measured by Preszler, et al.

  4. Monte-Carlo simulations of neutron-induced activation in a Fast-Neutron and Gamma-Based Cargo Inspection System

    NASA Astrophysics Data System (ADS)

    Bromberger, B.; Bar, D.; Brandis, M.; Dangendorf, V.; Goldberg, M. B.; Kaufmann, F.; Mor, I.; Nolte, R.; Schmiedel, M.; Tittelmeier, K.; Vartsky, D.; Wershofen, H.

    2012-03-01

    An air cargo inspection system combining two nuclear reaction based techniques, namely Fast-Neutron Resonance Radiography and Dual-Discrete-Energy Gamma Radiography is currently being developed. This system is expected to allow detection of standard and improvised explosives as well as special nuclear materials. An important aspect for the applicability of nuclear techniques in an airport inspection facility is the inventory and lifetimes of radioactive isotopes produced by the neutron radiation inside the cargo, as well as the dose delivered by these isotopes to people in contact with the cargo during and following the interrogation procedure. Using MCNPX and CINDER90 we have calculated the activation levels for several typical inspection scenarios. One example is the activation of various metal samples embedded in a cotton-filled container. To validate the simulation results, a benchmark experiment was performed, in which metal samples were activated by fast-neutrons in a water-filled glass jar. The induced activity was determined by analyzing the gamma spectra. Based on the calculated radioactive inventory in the container, the dose levels due to the induced gamma radiation were calculated at several distances from the container and in relevant time windows after the irradiation, in order to evaluate the radiation exposure of the cargo handling staff, air crew and passengers during flight. The possibility of remanent long-lived radioactive inventory after cargo is delivered to the client is also of concern and was evaluated.

  5. Rotation induced octupole correlations in the neutron-deficient 109Te nucleus

    NASA Astrophysics Data System (ADS)

    de Angelis, G.; Fahlander, C.; Gadea, A.; Farnea, E.; Bazzacco, D.; Belcari, N.; Blasi, N.; Bizzeti, P. G.; Bizzeti-Sona, A.; de Acuña, D.; de Poli, M.; Grawe, H.; Johnson, A.; Lo Bianco, G.; Lunardi, S.; Napoli, D. R.; Nyberg, J.; Pavan, P.; Persson, J.; Rossi Alvarez, C.; Rudolph, D.; Schubart, R.; Spolaore, P.; Wyss, R.; Xu, F.

    1998-10-01

    High spin states in the neutron deficient nucleus 109Te have been populated with the 58Ni+54Fe reaction at 220 MeV and investigated through γ-spectroscopy methods at the GASP spectrometer making use of reaction channel selection with the ISIS Si-ball. The level scheme has been extended up to an excitation energy of ~12.1 MeV. The spins and parities of the observed levels are assigned tentatively supporting the identification of two bands of opposite parity connected by strong dipole transitions inferred to be of E1 character. Octupole correlations in 109Te induced by rotation are suggested as the cause of this effect.

  6. Measurement of the 240,242Pu Neutron-induced Fission Cross Sections

    NASA Astrophysics Data System (ADS)

    Salvador-Castiñeira, P.; Bevilacqua, R.; Bryś, T.; Hambsch, F.-J.; Oberstedt, S.; Pretel, C.; Vidali, M.

    The neutron-induced fission cross section of 240,242Pu has been measured at the Van de Graaff facility of the Institute for Reference Materials and Measurements (JRC-IRMM). A Twin-Frisch Grid Ionization Chamber (TFGIC) has been used in a back-to-back geometry with the secondary standards 237Np and 238U to normalize the cross section. The energy range measured is from 0.2 keV up to 3 MeV. Preliminary results show some discrepancies around 1 MeV for the 242Pu with the ENDF/B-VII.1 evaluation. The spontaneous fission half-life has been measured for both isotopes, too. Preliminary results show reasonable agreement with the recommended values.

  7. Neutron scattering study of the field-induced tricritical point in MnSi

    NASA Astrophysics Data System (ADS)

    Kindervater, J.; Bauer, A.; Garst, M.; Janoschek, M.; Martin, N.; Mühlbauer, S.; Häussler, W.; Böni, P.; Pfleiderer, C.

    The intermetallic compound MnSi attracts great scientific interest due to two unusual phase transitions, namely the transition from the conical phase to a skyrmion lattice in small fields and the transition from the helical to the paramagnetic phase without external magnetic field that was recently identified to be a fluctuation induced first-order transition, i.e. a so called Brazovskii-transition. Recent measurements of the specific heat provide striking evidence for a tricritical point (TCP), were the first order transition alters to second order. We report neutron spin echo measurements using the MIEZE technique. The recorded quasi elastic linewidth shows a change of the characteristic spin fluctuations at the TCP. The combination with additional SANS measurements and a generalized Brazovskii theory establishes a consistent picture of the statics and dynamics of the transition. Financial support by ERC-AdG (291079 TOPFIT) and through DFG TRR80 is greatfully acknowledged.

  8. Neutron- and proton-induced reactions for analysis of bioenvironmental samples

    SciTech Connect

    Spyrou, N.M.; Altaf, W.J.; Khrbish, Y.S. )

    1988-01-01

    The study of the elemental composition of bioenvironmental samples is of continuing interest in a wide variety of medical and environmental investigations, be it as environmental monitors or as indicators of the state of health and disease of an individual or a population. Nuclear activation methods play an important role in these studies as research tools and in certain cases are employed as rapid, routine analytical techniques. Although the authors have been using instrumental neutron activation analysis as the main technique for obtaining information about elemental composition and concentration, they have also developed techniques, for further or complementary analysis, in which proton-induced reactions have been exploited. Two recent studies, in which the composition of human lung tissue and the elemental concentration in plant samples were determined, have been selected as illustrations of the techniques employed.

  9. Neutron yield and induced radioactivity: a study of 235-MeV proton and 3-GeV electron accelerators.

    PubMed

    Hsu, Yung-Cheng; Lai, Bo-Lun; Sheu, Rong-Jiun

    2016-01-01

    This study evaluated the magnitude of potential neutron yield and induced radioactivity of two new accelerators in Taiwan: a 235-MeV proton cyclotron for radiation therapy and a 3-GeV electron synchrotron serving as the injector for the Taiwan Photon Source. From a nuclear interaction point of view, neutron production from targets bombarded with high-energy particles is intrinsically related to the resulting target activation. Two multi-particle interaction and transport codes, FLUKA and MCNPX, were used in this study. To ensure prediction quality, much effort was devoted to the associated benchmark calculations. Comparisons of the accelerators' results for three target materials (copper, stainless steel and tissue) are presented. Although the proton-induced neutron yields were higher than those induced by electrons, the maximal neutron production rates of both accelerators were comparable according to their respective beam outputs during typical operation. Activation products in the targets of the two accelerators were unexpectedly similar because the primary reaction channels for proton- and electron-induced activation are (p,pn) and (γ,n), respectively. The resulting residual activities and remnant dose rates as a function of time were examined and discussed. PMID:25628454

  10. Neutron and Charged-Particle Induced Cross Sections for Radiochemistry in the Region of Samarium, Europium, and Gadolinium

    SciTech Connect

    Hoffman, R D; Kelley, K; Dietrich, F S; Bauer, R; Mustafa, M

    2004-11-30

    We have developed a set of modeled nuclear reaction cross sections for use in radiochemical diagnostics. Systematics for the input parameters required by the Hauser-Feshbach statistical model were developed and used to calculate neutron and proton induced nuclear reaction cross sections in the mass region of samarium, europium and gadolinium (62 {le} Z {le} 64, 82 {le} N {le} 96).

  11. Enrico Fermi's Discovery of Neutron-Induced Artificial Radioactivity:The Recovery of His First Laboratory Notebook

    NASA Astrophysics Data System (ADS)

    Acocella, Giovanni; Guerra, Francesco; Robotti, Nadia

    . We give a short description of the discovery of the first experimental notebook of Enrico Fermi (1901-1954) on his researches during March and April of 1934 on neutron-induced artificial radioactivity, and we point out its relevance for a proper historical and conceptual understanding of those researches.

  12. Revised Calculations of the Production Rates for Co Isotopes in Meteorites Using New Cross Sections for Neutron-induced Reactions

    NASA Technical Reports Server (NTRS)

    Sisterson, J. M.; Brooks, F. D.; Buffler, A.; Allie, M. S.; Herbert, M. S.; Nchodu, M. R.; Makupula, S.; Ullmann, J.; Reedy, R. C.; Jones, D. T. L.

    2002-01-01

    New cross section measurements for reactions induced by neutrons with energies greater than 70 MeV are used to calculate the production rates for cobalt isotopes in meteorites and these new calculations are compared to previous estimates. Additional information is contained in the original extended abstract.

  13. Neutron and Charged-Particle Induced Cross Sections for Radiochemistry in the Region of Bromine and Krypton

    SciTech Connect

    Hoffman, R; Dietrich, F; Bauer, R; Kelley, K; Mustafa, M

    2004-07-23

    We have developed a set of modeled nuclear reaction cross sections for use in radiochemical diagnostics. Systematics for the input parameters required by the Hauser-Feshbach statistical model were developed and used to calculate neutron and proton induced nuclear reaction cross sections in the mass region of bromine and krypton (34 {le} Z {le} 37, 40 {le} N {le} 47).

  14. Early stages of oxidative stress-induced membrane permeabilization: a neutron reflectometry study.

    PubMed

    Smith, Hillary L; Howland, Michael C; Szmodis, Alan W; Li, Qijuan; Daemen, Luke L; Parikh, Atul N; Majewski, Jaroslaw

    2009-03-18

    Neutron reflectometry was used to probe in situ the structure of supported lipid bilayers at the solid-liquid interface during the early stages of UV-induced oxidative degradation. Single-component supported lipid bilayers composed of gel phase, dipalmitoyl-sn-glycero-3-phosphocholine (DPPC), and fluid phase, 1-palmitoyl-2-oleoyl-sn-glycero-3-phosphocholine (POPC), phospholipids were exposed to low-dose oxidative stress generated by UV light and their structures were examined by neutron reflectometry. An interrupted illumination mode, involving exposures in 15 min increments with 2 h intervals between subsequent exposures, and a continuous mode involving a single 60 (or 90) min exposure period were employed. In both cases, pronounced differences in the structure of the lipid bilayer after exposure were observed. Interrupted exposure led to a substantial decrease in membrane coverage but preserved its total thickness at reduced scattering length densities. These results indicate that the initial phase during UV-induced membrane degradation involves the formation of hydrophilic channels within the membrane. This is consistent with the loss of some lipid molecules we observe and attendant reorganization of residual lipids forming hemimicellar edges of the hydrophilic channels. In contrast, continuous illumination produced a graded interface of continuously varied scattering length density (and hence hydrocarbon density) extending 100-150 A into the liquid phase. Exposure of a DPPC bilayer to UV light in the presence of a reservoir of unfused vesicles showed low net membrane disintegration during oxidative stress, presumably because of surface back-filling from the bulk reservoir. Chemical evidence for membrane degradation was obtained by mass spectrometry and Fourier transform infrared spectroscopy. Further evidence for the formation of hydrophilic channels was furnished by fluorescence microscopy and imaging ellipsometry data. PMID:19275260

  15. Early Stages of Oxidative Stress-Induced Membrane Permeabilization: A Neutron Reflectometry Study

    PubMed Central

    Smith, Hillary L.; Howland, Michael C.; Szmodis, Alan W.; Li, Qijuan; Daemen, Luke L.; Parikh, Atul N.; Majewski, Jaroslaw

    2009-01-01

    Neutron reflectometry was used to probe in situ the structure of supported lipid bilayers at the solid–liquid interface during the early stages of UV-induced oxidative degradation. Single-component supported lipid bilayers composed of gel phase, dipalmitoyl-sn-glycero-3-phosphocholine (DPPC), and fluid phase, 1-palmitoyl-2-oleoyl-sn-glycero-3-phosphocholine (POPC), phospholipids were exposed to low-dose oxidative stress generated by UV light and their structures were examined by neutron reflectometry. An interrupted illumination mode, involving exposures in 15 min increments with 2 h intervals between subsequent exposures, and a continuous mode involving a single 60 (or 90) min exposure period were employed. In both cases, pronounced differences in the structure of the lipid bilayer after exposure were observed. Interrupted exposure led to a substantial decrease in membrane coverage but preserved its total thickness at reduced scattering length densities. These results indicate that the initial phase during UV-induced membrane degradation involves the formation of hydrophilic channels within the membrane. This is consistent with the loss of some lipid molecules we observe and attendant reorganization of residual lipids forming hemimicellar edges of the hydrophilic channels. In contrast, continuous illumination produced a graded interface of continuously varied scattering length density (and hence hydrocarbon density) extending 100–150 Å into the liquid phase. Exposure of a DPPC bilayer to UV light in the presence of a reservoir of unfused vesicles showed low net membrane disintegration during oxidative stress, presumably because of surface back-filling from the bulk reservoir. Chemical evidence for membrane degradation was obtained by mass spectrometry and Fourier transform infrared spectroscopy. Further evidence for the formation of hydrophilic channels was furnished by fluorescence microscopy and imaging ellipsometry data. PMID:19275260

  16. RhG-CSF improves radiation-induced myelosuppression and survival in the canine exposed to fission neutron irradiation.

    PubMed

    Yu, Zu-Yin; Li, Ming; Han, A-Ru-Na; Xing, Shuang; Ou, Hong-Ling; Xiong, Guo-Lin; Xie, Ling; Zhao, Yan-Fang; Xiao, He; Shan, Ya-Jun; Zhao, Zhen-Hu; Liu, Xiao-Lan; Cong, Yu-Wen; Luo, Qing-Liang

    2011-01-01

    Fission-neutron radiation damage is hard to treat due to its critical injuries to hematopoietic and gastrointestinal systems, and so far few data are available on the therapeutic measures for neutron-radiation syndrome. This study was designed to test the effects of recombinant human granulocyte colony-stimulating factor (rhG-CSF) in dogs which had received 2.3 Gy mixed fission-neutron-γ irradiation with a high ratio of neutrons (~90%). Following irradiation, rhG-CSF treatment induced 100% survival versus 60% in controls. Only two of five rhG-CSF-treated dogs experienced leukopenia (white blood cells [WBC] count < 1.0 × 10(9)/L) and neutropenia (neutrophil [ANC] count < 0.5 × 10(9)/L), whereas all irradiated controls displayed a profound period of leukopenia and neutropenia. Furthermore, administration of rhG-CSF significantly delayed the onset of leukopenia and reduced the duration of leucopenia as compared with controls. In addition, individual dogs in the rhG-CSF-treated group exhibited evident differences in rhG-CSF responsiveness after neutron-irradiation. Finally, histopathological evaluation of the surviving dogs revealed that the incidence and severity of bone marrow, thymus and spleen damage decreased in rhG-CSF-treated dogs as compared with surviving controls. Thus, these results demonstrated that rhG-CSF administration enhanced recovery of myelopoiesis and survival after neutron-irradiation. PMID:21785235

  17. TANGRA-Setup for the Investigation of Nuclear Fission Induced by 14.1 MeV Neutrons

    NASA Astrophysics Data System (ADS)

    Ruskov, I. N.; Kopatch, Yu. N.; Bystritsky, V. M.; Skoy, V. R.; Shvetsov, V. N.; Hambsch, F.-J.; Oberstedt, S.; Noy, R. Capote; Sedyshev, P. V.; Grozdanov, D. N.; Ivanov, I. Zh.; Aleksakhin, V. Yu.; Bogolubov, E. P.; Barmakov, Yu. N.; Khabarov, S. V.; Krasnoperov, A. V.; Krylov, A. R.; Obhođaš, J.; Pikelner, L. B.; Rapatskiy, V. L.; Rogachev, A. V.; Rogov, Yu. N.; Ryzhkov, V. I.; Sadovsky, A. B.; Salmin, R. A.; Sapozhnikov, M. G.; Slepnev, V. M.; Sudac, D.; Tarasov, O. G.; Valković, V.; Yurkov, D. I.; Zamyatin, N. I.; Zeynalov, Sh. S.; Zontikov, A. O.; Zubarev, E. V.

    The new experimental setup TANGRA (Tagged Neutrons & Gamma Rays), for the investigation of neutron induced nuclear reactions, e.g. (n,xn'), (n,xn'γ), (n,γ), (n,f), on a number of important isotopes for nuclear science and engineering (235,238U, 237Np, 239Pu, 244,245,248Cm) is under construction and being tested at the Frank Laboratory of Neutron Physics (FLNP) of the Joint Institute for Nuclear Research (JINR) in Dubna. The TANGRA setup consists of: a portable neutron generator ING-27, with a 64-pixel Si charge-particle detector incorporated into its vacuum chamber for registering of α-particles formed in the T(d, n)4He reaction, as a source of 14.1 MeV steady-state neutrons radiation with an intensity of ∼5x107n/s; a combined iron (Fe), borated polyethylene (BPE) and lead (Pb) compact shielding-collimator; a reconfigurable multi-detector (neutron plus gamma ray detecting system); a fast computer with 2 (x16 channels) PCI-E 100 MHz ADC cards for data acquisition and hard disk storage; Linux ROOT data acquisition, visualization and analysis software. The signals from the α-particle detector are used to 'tag' the neutrons with the coincident α-particles. Counting the coincidences between the α-particle and the reaction-product detectors in a 20ns time-interval improves the effect/background-ratio by a factor of ∼200 as well as the accuracy in the neutron flux determination, which decreases noticeably the overall experimental data uncertainty.

  18. Thermal neutron imaging in an active interrogation environment

    SciTech Connect

    Vanier,P.E.; Forman, L., and Norman, D.R.

    2009-03-10

    We have developed a thermal-neutron coded-aperture imager that reveals the locations of hydrogenous materials from which thermal neutrons are being emitted. This imaging detector can be combined with an accelerator to form an active interrogation system in which fast neutrons are produced in a heavy metal target by means of xcitation by high energy photons. The photo-induced neutrons can be either prompt or delayed, depending on whether neutronemitting fission products are generated. Provided that there are hydrogenous materials close to the target, some of the photo-induced neutrons slow down and emerge from the surface at thermal energies. These neutrons can be used to create images that show the location and shape of the thermalizing materials. Analysis of the temporal response of the neutron flux provides information about delayed neutrons from induced fission if there are fissionable materials in the target. The combination of imaging and time-of-flight discrimination helps to improve the signal-to-background ratio. It is also possible to interrogate the target with neutrons, for example using a D-T generator. In this case, an image can be obtained from hydrogenous material in a target without the presence of heavy metal. In addition, if fissionable material is present in the target, probing with fast neutrons can stimulate delayed neutrons from fission, and the imager can detect and locate the object of interest, using appropriate time gating. Operation of this sensitive detection equipment in the vicinity of an accelerator presents a number of challenges, because the accelerator emits electromagnetic interference as well as stray ionizing radiation, which can mask the signals of interest.

  19. Neutron-induced fission cross section of 233Pa between 1.0 and 3.0 MeV.

    PubMed

    Tovesson, F; Hambsch, F J; Oberstedt, A; Fogelberg, B; Ramström, E; Oberstedt, S

    2002-02-11

    The energy dependent neutron-induced fission cross section of 233Pa has for the first time been measured directly with monoenergetic neutrons. This nuclide is an important intermediary in a thorium based fuel cycle, and its fission cross section is a key parameter in the modeling of future advanced fuel and reactor concepts. A first experiment resulted in four cross section values between 1.0 and 3.0 MeV, establishing a fission threshold in excess of 1 MeV. Significant discrepancies were found with a previous indirect experimental determination and with model estimates. PMID:11863801

  20. Energy dependence of mass, charge, isotopic, and energy distributions in neutron-induced fission of 235U and 239Pu

    NASA Astrophysics Data System (ADS)

    Pasca, H.; Andreev, A. V.; Adamian, G. G.; Antonenko, N. V.; Kim, Y.

    2016-05-01

    The mass, charge, isotopic, and kinetic-energy distributions of fission fragments are studied within an improved scission-point statistical model in the reactions 235U+n and 239Pu+n at different energies of the incident neutron. The charge and mass distributions of the electromagnetic- and neutron-induced fission of 214,218Ra, 230,232,238U are also shown. The available experimental data are well reproduced and the energy-dependencies of the observable characteristics of fission are predicted for future experiments.

  1. 78 FR 5450 - Information Collection; Prompt Payment

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-01-25

    ... GENERAL SERVICES ADMINISTRATION NATIONAL AERONAUTICS AND SPACE ADMINISTRATION Information Collection... and approve an extension to a previously approved information collection requirement concerning prompt... Information Collection 9000- 0102, Prompt Payment, by any of the following methods: Regulations.gov :...

  2. Neutron scattering studies in the actinide region. Progress report, August 1, 1991--July 31, 1994

    SciTech Connect

    Kegel, G.H.R.; Egan, J.J.

    1994-09-01

    During the period August 1, 1991 to July 31, 1994 the authors report progress on the following: (a) prompt fission neutron energy spectra for {sup 235}U and {sup 239}Pu; (b) two-parameter measurement of nuclear lifetimes; (c) `black` neutron detector; (d) data reduction techniques for neutron scattering experiments; (e) elastic and inelastic neutron scattering studies in {sup 197}Au; (f) elastic and inelastic neutron scattering studies in {sup 239}Pu; (g) neutron induced defects in silicon dioxide MOS structures; (h) response of a {sup 235}U fission chamber near reaction thresholds; (i) efficiency calibration of a liquid scintillation detector using the WNR facility at LAMPF; (j) prompt fission neutron energy spectrum measurements below the incident neutron energy; (k) multi-parameter data acquisition system; (l) accelerator improvements; (m) non-DOE supported research. Eight Ph.D. dissertations and two M.S. theses were completed during the report period. Publications consisted of 6 journal articles, 10 conference proceedings, and 19 abstracts of presentations at scientific meetings. One invited talk was given.

  3. Proteomic analysis of cellular response induced by boron neutron capture reaction in human squamous cell carcinoma SAS cells.

    PubMed

    Sato, Akira; Itoh, Tasuku; Imamichi, Shoji; Kikuhara, Sota; Fujimori, Hiroaki; Hirai, Takahisa; Saito, Soichiro; Sakurai, Yoshinori; Tanaka, Hiroki; Nakamura, Hiroyuki; Suzuki, Minoru; Murakami, Yasufumi; Baiseitov, Diaz; Berikkhanova, Kulzhan; Zhumadilov, Zhaxybay; Imahori, Yoshio; Itami, Jun; Ono, Koji; Masunaga, Shinichiro; Masutani, Mitsuko

    2015-12-01

    To understand the mechanism of cell death induced by boron neutron capture reaction (BNCR), we performed proteome analyses of human squamous tumor SAS cells after BNCR. Cells were irradiated with thermal neutron beam at KUR after incubation under boronophenylalanine (BPA)(+) and BPA(-) conditions. BNCR mainly induced typical apoptosis in SAS cells 24h post-irradiation. Proteomic analysis in SAS cells suggested that proteins functioning in endoplasmic reticulum, DNA repair, and RNA processing showed dynamic changes at early phase after BNCR and could be involved in the regulation of cellular response to BNCR. We found that the BNCR induces fragments of endoplasmic reticulum-localized lymphoid-restricted protein (LRMP). The fragmentation of LRMP was also observed in the rat tumor graft model 20 hours after BNCT treatment carried out at the National Nuclear Center of the Republic of Kazakhstan. These data suggest that dynamic changes of LRMP could be involved during cellular response to BNCR. PMID:26302661

  4. Measurements of Neutron-Induced Fission Cross Sections of 205Tl, 204, 206, 207, 208Pb, and 209Bi using Quasi-Monoenergetic Neutrons in the Energy Range 35 - 174 MeV

    NASA Astrophysics Data System (ADS)

    Tutin, Gennady A.; Ryzhov, Igor V.; Eismont, Vilen P.; Mitryukhin, Andrey G.; Oplavin, Valery S.; Soloviev, Sergey M.; Blomgren, Jan; Condè, Henri; Olsson, Nils; Renberg, Per-Ulf

    2005-05-01

    Cross sections for neutron-induced fission of 205Tl, 204, 206, 207, 208Pb, and 209Bi were measured in the energy range from 35 MeV to 174 MeV. The experiments were done at the neutron beam facility of The Svedberg Laboratory, using a multi-section Frisch-gridded ionization chamber for detection of the fission fragments. The neutron-induced fission cross section of 238U was employed as a reference. The results of the measurements are compared with existing experimental data.

  5. Method for on-line evaluation of materials using prompt gamma ray analysis

    DOEpatents

    Akers, Douglas W.

    2009-12-08

    A method for evaluating a material specimen comprises: Mounting a neutron source and a detector adjacent the material specimen; bombarding the material specimen with neutrons from the neutron source to create prompt gamma rays within the material specimen, some of the prompt gamma rays being emitted from the material specimen, some of the prompt gamma rays resulting in the formation of positrons within the material specimen by pair production; collecting positron annihilation data by detecting with the detector at least one emitted annihilation gamma ray resulting from the annihilation of a positron; storing the positron annihilation data on a data storage system for later retrieval and processing; and continuing to collect and store positron annihilation data, the continued collected and stored positron annihilation data being indicative of an accumulation of lattice damage over time.

  6. Of mermaids and mountains. Three decades of prompt activation in vivo.

    PubMed

    Morgan, W D

    2000-05-01

    During 1966 to 1972, several laboratories demonstrated the feasibility of measuring the major body elements H, N, Ca, and Cl by prompt gamma in vivo neutron activation analysis (PGIVNA). The MERMAID facility in Birmingham, England used a cyclotron-produced pulsed neutron beam, but other groups in the United Kingdom, United States, Canada, and New Zealand subsequently developed systems based on radioisotope neutron sources that could measure body nitrogen with a precision of a margin of error of a few percentage points. The accuracy of N measurement was greatly enhanced by Vartsky's internal standardization, using prompt-gamma H as the marker and total body hydrogen (based on total body water and skinfolds) as the reference. Chlorine and extracellular water volume were used in a similar way by the Swansea group to calibrate the prompt-gamma analysis of total body calcium. The PGIVNA technique is most valuable in assessing nutritional status, particularly in relation to body protein. PMID:10865724

  7. WE-D-BRF-03: Proton Beam Range Verification with a Single Prompt Gamma-Ray Detector

    SciTech Connect

    Verburg, J; Testa, M; Cascio, E; Bortfeld, T; Lu, H; Seco, J

    2014-06-15

    Purpose: To present an experimental study of a novel range verification method for scanned and scattered proton beams. Methods: A detection system consisting of an actively shielded lanthanum(III)bromide scintillator and a one-sided lead collimator was used to measure prompt gamma-rays emitted during the delivery of proton beams to a water phantom and an anthropomorphic head phantom. The residual proton range at the collimator position was determined by comparing gamma-ray intensities while the proton energy was modulated to the distal end of the target. We used a clinical field to deliver a 50 cGy dose to a 12 cm diameter target in the water phantom and to a 175 cc tumor-shaped target in the head phantom. The detector signals were acquired with a custom data acquisition system enabling energy and time-of-flight discrimination of prompt gamma-rays. Results: Range deviations were detected with a statistical accuracy of ± 0.2 mm and ± 1.4 mm at 90% confidence level, respectively for the water and head phantom. We obtained a time resolution of 1 ns FWHM and an energy resolution < 2% FWHM for the main gamma lines from proton-induced nuclear reactions with carbon and oxygen. This allowed for an accurate separation of the prompt gamma-rays from neutron-induced background. Conclusion: Proton range deviations can be detected with millimeter accuracy using a single prompt gamma-ray measurement point acquired during the delivery of a few proton energy layers to the distal part of the target. The method is also feasible in the presence of background radiation from passively scattered proton beam delivery.

  8. 38 CFR 1.950 - Prompt referral.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 38 Pensions, Bonuses, and Veterans' Relief 1 2010-07-01 2010-07-01 false Prompt referral. 1.950 Section 1.950 Pensions, Bonuses, and Veterans' Relief DEPARTMENT OF VETERANS AFFAIRS GENERAL PROVISIONS Referrals to Gao, Department of Justice, Or Irs § 1.950 Prompt referral. (a) VA shall promptly refer...

  9. 38 CFR 1.950 - Prompt referral.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 38 Pensions, Bonuses, and Veterans' Relief 1 2011-07-01 2011-07-01 false Prompt referral. 1.950 Section 1.950 Pensions, Bonuses, and Veterans' Relief DEPARTMENT OF VETERANS AFFAIRS GENERAL PROVISIONS Referrals to Gao, Department of Justice, Or Irs § 1.950 Prompt referral. (a) VA shall promptly refer...

  10. Determination of neutron-induced alpha-particle cross sections on carbon using the response of a liquid scintillation detector

    SciTech Connect

    Brede, H.J.; Dietze, G.; Klein, H.; Schoelermann, H. )

    1991-01-01

    This paper presents the sums of the cross section {sup 12}C(n, {alpha}{sub 0}) {sup 9}Be and {sup 12}C(n, N{prime}3{alpha}) determined in the neutron energy range between 7.4 and 11 MeV. An NE-213 scintillation detector is simultaneously used as a carbon target, an alpha-particle detector, and a neutron fluence monitor. By comparing the measured and calculated response spectra, the neutron-induced alpha-particle events in the scintillation volume are separated and the cross sections {sigma}{sub n,{alpha}0} + {sigma}{sub n,n{prime}3{alpha}} are determined relative to the n-p scattering cross section. The pulse-height distribution due to alpha particles allows the angular distribution to be extracted on the basis of the reaction kinematics and an accurately determined light output function for alpha particles in the NE-213 detector.

  11. Range verification of passively scattered proton beams using prompt gamma-ray detection

    NASA Astrophysics Data System (ADS)

    Verburg, Joost M.; Testa, Mauro; Seco, Joao

    2015-02-01

    We performed an experimental study to verify the range of passively scattered proton beams by detecting prompt gamma-rays emitted from proton-nuclear interactions. A method is proposed using a single scintillation detector positioned near the distal end of the irradiated target. Lead shielding was used to attenuate gamma-rays emitted along most of the entrance path of the beam. By synchronizing the prompt gamma-ray detector to the rotation of the range modulation wheel, the relation between the gamma emission from the distal part of the target and the range of the incident proton beam was determined. In experiments with a water phantom and an anthropomorphic head phantom, this relation was found to be sensitive to range shifts that were introduced. The wide opening angle of the detector enabled a sufficient signal-to-background ratio to be achieved in the presence of neutron-induced background from the scattering and collimating devices. Uniform range shifts were detected with a standard deviation of 0.1 mm to 0.2 mm at a dose level of 30 cGy to 50 cGy (RBE). The detectable magnitude of a range shift limited to a part of the treatment field area was approximately proportional to the ratio between the field area and the area affected by the range shift. We conclude that it is feasible to detect changes in the range of passively scattered proton beams using a relatively simple prompt gamma-ray detection system. The method can be employed for in vivo verification of the consistency of the delivered range in fractionated treatments.

  12. Characterization of neutron induced damage effect in several types of metallic multilayer nanocomposites based on Monte Carlo simulation

    NASA Astrophysics Data System (ADS)

    Chen, Feida; Tang, Xiaobin; Yang, Yahui; Huang, Hai; Liu, Jian; Chen, Da

    2015-09-01

    Metallic multilayer nanocomposites are known to have excellent interface self-healing performance when it comes to repairing irradiation damages, thus showing promise as structural materials for advanced nuclear power systems. The present study investigated the neutron irradiation displacement damage rate, spectra of the primary knocked-on atoms (PKAs) produced in the cascade collision, and the H/He ratio in four kinds of metallic multilayer nanocomposites (Cu/Nb, Ag/V, Fe/W, and Ti/Ta) versus neutrons' energy. Results suggest that the three neutron induced damage effects in all multilayer systems increased with the increasing of incident neutrons' energy. For fission reactor environment (1 MeV), multilayer's displacement damage rate is 5-10 × 1022 dpa/(n/cm2) and the mean PKAs energy is about 16 keV, without any noteworthy H/He produced. Fe/W multilayer seems very suitable among these four systems. For fusion reactor environment (14 MeV), the dominant damage effect varies in different multilayer systems. Fe/W multilayer has the lowest displacement damage under the same neutron flux but its gaseous transmutation production is the highest. Considering the displacement damage and transmutation, the irradiation resistance of Ag/V and Ti/Ta systems seems much greater than those of the other two.

  13. Moisture effect in prompt gamma measurements from soil samples.

    PubMed

    Naqvi, A A; Khiari, F Z; Liadi, F A; Khateeb-Ur-Rehman; Raashid, M A; Isab, A H

    2016-09-01

    The variation in intensity of 1.78MeV silicon, 6.13MeV oxygen, and 2.22MeV hydrogen prompt gamma rays from soil samples due to the addition of 5.1, 7.4, 9.7, 11.9 and 14.0wt% water was studied for 14MeV incident neutron beams utilizing a LaBr3:Ce gamma ray detector. The intensities of 1.78MeV and 6.13MeV gamma rays from silicon and oxygen, respectively, decreased with increasing sample moisture. The intensity of 2.22MeV hydrogen gamma rays increases with moisture. The decrease in intensity of silicon and oxygen gamma rays with moisture concentration indicates a loss of 14MeV neutron flux, while the increase in intensity of 2.22MeV gamma rays with moisture indicates an increase in thermal neutron flux due to increasing concentration of moisture. The experimental intensities of silicon, oxygen and hydrogen prompt gamma rays, measured as a function of moisture concentration in the soil samples, are in good agreement with the theoretical results obtained through Monte Carlo calculations. PMID:27337651

  14. Prompt fission γ -ray spectrum characteristics from 240Pu(sf ) and 242Pu(sf )

    NASA Astrophysics Data System (ADS)

    Oberstedt, S.; Oberstedt, A.; Gatera, A.; Göök, A.; Hambsch, F.-J.; Moens, A.; Sibbens, G.; Vanleeuw, D.; Vidali, M.

    2016-05-01

    In this paper we present first results for prompt fission γ -ray spectra (PFGS) characteristics from the spontaneous fission (sf) of 240Pu and 242Pu. For 242Pu(sf ) we obtained, after proper unfolding of the detector response, an average energy per photon ɛ¯γ=(0.843 ±0.012 ) MeV, an average multiplicity M¯γ=(6.72 ±0.07 ) , and an average total γ -ray energy release per fission E¯γ ,tot = (5.66 ± 0.06) MeV. The 240Pu(sf ) emission spectrum was obtained by applying a so-called detector-response transformation function determined from the 242Pu spectrum measured in exactly the same geometry. The results are an average energy per photon ɛ¯γ=(0.80 ±0.07 ) MeV, the average multiplicity M¯γ = (8.2 ± 0.4), and an average total γ -ray energy release per fission E¯γ ,tot = (6.6 ± 0.5) MeV. The PFGS characteristics for 242Pu(sf ) are in very good agreement with those from thermal-neutron-induced fission on 241Pu and scales well with the corresponding prompt neutron multiplicity. Our results in the case of 240Pu(sf ), although drawn from a limited number of events, show a significantly enhanced average multiplicity and average total energy, but may be understood from a different fragment yield distribution in 240Pu(sf ) compared to that of 242Pu(sf ).

  15. Neutron triples counting data for uranium

    NASA Astrophysics Data System (ADS)

    Croft, Stephen; LaFleur, Adrienne M.; McElroy, Robert D.; Swinhoe, Martyn T.

    2015-06-01

    Correlated neutron counting using multiplicity shift register logic extracts the first three factorial moments from the detected neutron pulse train. The descriptive properties of the measurement item (mass, the ratio of (α,n) to spontaneous fission neutron production, and leakage self-multiplication) are related to the observed singles (S), doubles (D) and triples (T) rates, and this is the basis of the widely used multiplicity counting assay method. The factorial moments required to interpret and invert the measurement data in the framework of the point kinetics model may be calculated from the spontaneous fission prompt neutron multiplicity distribution P(ν). In the case of 238U very few measurements of P(ν) are available and the derived values, especially for the higher factorial moments, are not known with high accuracy. In this work, we report the measurement of the triples rate per gram of 238U based on the analysis of a set of measurements in which a collection of 10 cylinders of UO2F2, each containing about 230 g of compound, were measured individually and in groups. Special care was taken to understand and compensate the recorded multiplicity histograms for the effect of random cosmic-ray induced background neutrons, which, because they also come in bursts and mimic fissions but with a different and harder multiplicity distribution. We compare our fully corrected (deadtime, background, efficiency, multiplication) experimental results with first principles expectations based on evaluated nuclear data. Based on our results we suspect that the current evaluated nuclear data is biased, which points to a need to undertake new basic measurements of the 238U prompt neutron multiplicity distribution.

  16. Prompting technologies: A comparison of time-based and context-aware transition-based prompting

    PubMed Central

    Robertson, Kayela; Rosasco, Cody; Feuz, Kyle; Schmitter-Edgecombe, Maureen; Cook, Diane

    2016-01-01

    BACKGROUND While advancements in technology have encouraged the development of novel prompting systems to support cognitive interventions, little research has evaluated the best time to deliver prompts, which may impact the effectiveness of these interventions. OBJECTIVE This study examined whether transition-based context prompting (prompting an individual during task transitions) is more effective than traditional fixed time-based prompting. METHODS Participants were 42 healthy adults who completed 12 different everyday activities, each lasting 1–7 minutes, in an experimental smart home testbed and received prompts to record the completed activities from an electronic memory notebook. Half of the participants were delivered prompts during activity transitions, while the other half received prompts every 5 minutes. Participants also completed Likert-scale ratings regarding their perceptions of the prompting system. RESULTS Results revealed that participants in the transition-based context prompting condition responded to the first prompt more frequently and rated the system as more convenient, natural, and appropriate compared to participants in the time-based condition. CONCLUSIONS Our findings suggest that prompting during activity transitions produces higher adherence to the first prompt and more positive perceptions of the prompting system. This is an important finding given the benefits of prompting technology and the possibility of improving cognitive interventions by using context-aware transition prompting. PMID:26409520

  17. Boron neutron capture therapy induces cell cycle arrest and cell apoptosis of glioma stem/progenitor cells in vitro

    PubMed Central

    2013-01-01

    Background Glioma stem cells in the quiescent state are resistant to clinical radiation therapy. An almost inevitable glioma recurrence is due to the persistence of these cells. The high linear energy transfer associated with boron neutron capture therapy (BNCT) could kill quiescent and proliferative cells. Methods The present study aimed to evaluate the effects of BNCT on glioma stem/progenitor cells in vitro. The damage induced by BNCT was assessed using cell cycle progression, apoptotic cell ratio and apoptosis-associated proteins expression. Results The surviving fraction and cell viability of glioma stem/progenitor cells were decreased compared with differentiated glioma cells using the same boronophenylalanine pretreatment and the same dose of neutron flux. BNCT induced cell cycle arrest in the G2/M phase and cell apoptosis via the mitochondrial pathway, with changes in the expression of associated proteins. Conclusions Glioma stem/progenitor cells, which are resistant to current clinical radiotherapy, could be effectively killed by BNCT in vitro via cell cycle arrest and apoptosis using a prolonged neutron irradiation, although radiosensitivity of glioma stem/progenitor cells was decreased compared with differentiated glioma cells when using the same dose of thermal neutron exposure and boronophenylalanine pretreatment. Thus, BNCT could offer an appreciable therapeutic advantage to prevent tumor recurrence, and may become a promising treatment in recurrent glioma. PMID:23915425

  18. Measurements and analyses of decay radioactivity induced in simulated deuterium-tritium neutron environments for fusion reactor structural materials

    SciTech Connect

    Ikeda, Y.; Konno, C.; Kosako, K.; Oyama, Y.; Maekawa, F.; Maekawa, H.; Kumar, A.; Youssef, M.Z.; Abdou, M.A.

    1995-08-01

    To meet urgent requirements for data validation, an experimental analysis has been carried out for isotopic radioactivity induced by deuterium-tritium neutron irradiation in structural materials. The primary objective is to examine the adequacy of the activation cross sections implemented in the current activation calculation codes considered for use in fusion reactor nuclear design. Four activation cross-section libraries, namely, JENDL, LIB90, REAC{sup *}63, and REAC{sup *}175 were investigated in this current analysis. The isotopic induced radioactivity calculations using these four libraries are compared with experimental values obtained in the Japan Atomic Energy Research Institute/U.S. Department of Energy collaborative program on fusion blanket neutronics. The nine materials studied are aluminum, silicon, titanium, vanadium, chromium, MnCu alloy, iron, nickel, niobium, and Type 316 stainless steel. The adequacy of the cross sections is investigated through the calculation to experiment analysis. As a result, most of the discrepancies in the calculations from experiments can be explained by inadequate activation cross sections. In addition, uncertainties due to neutron energy groups and neutron transport calculation are considered. The JENDL library gives the best agreement with experiments, followed by REAC{sup *}175, LIB90, and REAC{sup *}63, in this order. 45 refs., 32 figs., 5 tabs.

  19. Prompt gamma-ray imaging for small animals

    NASA Astrophysics Data System (ADS)

    Xu, Libai

    Small animal imaging is recognized as a powerful discovery tool for small animal modeling of human diseases, which is providing an important clue to complete understanding of disease mechanisms and is helping researchers develop and test new treatments. The current small animal imaging techniques include positron emission tomography (PET), single photon emission tomography (SPECT), computed tomography (CT), magnetic resonance imaging (MRI), and ultrasound (US). A new imaging modality called prompt gamma-ray imaging (PGI) has been identified and investigated primarily by Monte Carlo simulation. Currently it is suggested for use on small animals. This new technique could greatly enhance and extend the present capabilities of PET and SPECT imaging from ingested radioisotopes to the imaging of selected non-radioactive elements, such as Gd, Cd, Hg, and B, and has the great potential to be used in Neutron Cancer Therapy to monitor neutron distribution and neutron-capture agent distribution. This approach consists of irradiating small animals in the thermal neutron beam of a nuclear reactor to produce prompt gamma rays from the elements in the sample by the radiative capture (n, gamma) reaction. These prompt gamma rays are emitted in energies that are characteristic of each element and they are also produced in characteristic coincident chains. After measuring these prompt gamma rays by surrounding spectrometry array, the distribution of each element of interest in the sample is reconstructed from the mapping of each detected signature gamma ray by either electronic collimations or mechanical collimations. In addition, the transmitted neutrons from the beam can be simultaneously used for very sensitive anatomical imaging, which provides the registration for the elemental distributions obtained from PGI. The primary approach is to use Monte Carlo simulation methods either with the specific purpose code CEARCPG, developed at NC State University or with the general purpose

  20. Production, distribution and applications of californium-252 neutron sources.

    PubMed

    Martin, R C; Knauer, J B; Balo, P A

    2000-01-01

    The radioisotope 252Cf is routinely encapsulated into compact, portable, intense neutron sources with a 2.6-yr half-life. A source the size of a person's little finger can emit up to 10(11) neutrons s(-1). Californium-252 is used commercially as a reliable, cost-effective neutron source for prompt gamma neutron activation analysis (PGNAA) of coal, cement and minerals, as well as for detection and identification of explosives, land mines and unexploded military ordinance. Other uses are neutron radiography, nuclear waste assays, reactor start-up sources, calibration standards and cancer therapy. The inherent safety of source encapsulations is demonstrated by 30 yr of experience and by US Bureau of Mines tests of source survivability during explosions. The production and distribution center for the US Department of Energy (DOE) Californium Program is the Radiochemical Engineering Development Center (REDC) at Oak Ridge National Laboratory (ORNL). DOE sells 252Cf to commercial reencapsulators domestically and internationally. Sealed 252Cf sources are also available for loan to agencies and subcontractors of the US government and to universities for educational, research and medical applications. The REDC has established the Californium User Facility (CUF) for Neutron Science to make its large inventory of 252Cf sources available to researchers for irradiations inside uncontaminated hot cells. Experiments at the CUF include a land mine detection system, neutron damage testing of solid-state detectors, irradiation of human cancer cells for boron neutron capture therapy experiments and irradiation of rice to induce genetic mutations. PMID:11003521

  1. Neutron reflectometry on highly absorbing films and its application to 10B4C-based neutron detectors

    PubMed Central

    Piscitelli, F.; Khaplanov, A.; Devishvili, A.; Schmidt, S.; Höglund, C.; Birch, J.; Dennison, A. J. C.; Gutfreund, P.; Hall-Wilton, R.; Van Esch, P.

    2016-01-01

    Neutron reflectometry is a powerful tool used for studies of surfaces and interfaces. The absorption in the typical studied materials is neglected and this technique is limited only to the reflectivity measurement. For strongly absorbing nuclei, the absorption can be directly measured by using the neutron-induced fluorescence technique which exploits the prompt particle emission of absorbing isotopes. This technique is emerging from soft matter and biology where highly absorbing nuclei, in very small quantities, are used as a label for buried layers. Nowadays, the importance of absorbing layers is rapidly increasing, partially because of their application in neutron detection; a field that has become more active also due to the 3He-shortage. We extend the neutron-induced fluorescence technique to the study of layers of highly absorbing materials, in particular 10B4C. The theory of neutron reflectometry is a commonly studied topic; however, when a strong absorption is present the subtle relationship between the reflection and the absorption of neutrons is not widely known. The theory for a general stack of absorbing layers has been developed and compared to measurements. We also report on the requirements that a 10B4C layer must fulfil in order to be employed as a converter in neutron detection. PMID:26997902

  2. Particular features of ternary fission induced by polarized neutrons in the major actinides U,235233 and Pu,241239

    NASA Astrophysics Data System (ADS)

    Gagarski, A.; Gönnenwein, F.; Guseva, I.; Jesinger, P.; Kopatch, Yu.; Kuzmina, T.; Lelièvre-Berna, E.; Mutterer, M.; Nesvizhevsky, V.; Petrov, G.; Soldner, T.; Tiourine, G.; Trzaska, W. H.; Zavarukhina, T.

    2016-05-01

    Ternary fission in (n ,f ) reactions was studied with polarized neutrons for the isotopes U,235233 and Pu,241239. A cold longitudinally polarized neutron beam was available at the High Flux Reactor of the Institut Laue-Langevin in Grenoble, France. The beam was hitting the fissile targets mounted at the center of a reaction chamber. Detectors for fission fragments and ternary particles were installed in a plane perpendicular to the beam. In earlier work it was discovered that the angular correlations between neutron spin and the momenta of fragments and ternary particles were very different for 233U or 235U. These correlations could now be shown to be simultaneously present in all of the above major actinides though with different weights. For one of the correlations it was observed that up to scission the compound nucleus is rotating with the axis of rotation parallel to the neutron beam polarization. Entrained by the fragments also the trajectories of ternary particles are turned away albeit by a smaller angle. The difference in turning angles becomes observable upon reversing the sense of rotation by flipping neutron spin. All turning angles are smaller than 1∘. The phenomenon was called the ROT effect. As a distinct second phenomenon it was found that for fission induced by polarized neutrons an asymmetry in the emission probability of ternary particles relative to a plane formed by fragment momentum and neutron spin appears. The asymmetry is attributed to the Coriolis force present in the nucleus while it is rotating up to scission. The size of the asymmetry is typically 10-3. This asymmetry was termed the TRI effect. The interpretation of both effects is based on the transition state model. Both effects are shown to be steered by the properties of the collective (J ,K ) transition states which are specific for any of the reactions studied. The study of asymmetries of ternary particle emission in fission induced by slow polarized neutrons provides a new

  3. Genetic effects induced by neutrons in Drosophila melanogaster I. Determination of absorbed dose.

    PubMed

    Delfin, A; Paredes, L C; Zambrano, F; Guzmán-Rincón, J; Ureña-Nuñez, F

    2001-12-01

    A method to obtain the absorbed dose in Drosophila melanogaster irradiated in the thermal column facility of the Triga Mark III Reactor has been developed. The method is based on the measurements of neutron activation of gold foils produced by neutron capture to obtain the neutron fluxes. These fluxes, combined with the calculations of kinetic energy released per unit mass, enables one to obtain the absorbed doses in Drosophila melanogaster. PMID:11761104

  4. Towards high accurate neutron-induced fission cross sections of 240,242Pu: Spontaneous fission half-lives

    NASA Astrophysics Data System (ADS)

    Salvador-Castiñeira, P.; Bryś, T.; Eykens, R.; Hambsch, F.-J.; Moens, A.; Oberstedt, S.; Pretel, C.; Sibbens, G.; Vanleeuw, D.; Vidali, M.

    2013-12-01

    Fast spectrum neutron-induced fission cross sections of transuranic isotopes are being of special demand in order to provide accurate data for the new GEN-IV nuclear power plants. To minimize the uncertainties on these measurements accurate data on spontaneous fission half-lives and detector efficiencies are a key point. High α-active actinides need special attention since the misinterpretation of detector signals can lead to low efficiency values or underestimation in fission fragment detection. In that context, 240,242Pu isotopes have been studied by means of a Twin Frisch-Grid Ionization Chamber (TFGIC) for measurements of their neutron-induced fission cross section. Gases with different drift velocities have been used, namely P10 and CH4. The detector efficiencies for both samples have been determined and improved spontaneous fission half-life values were obtained.

  5. Background Neutron Studies for Coherent Elastic Neutrino-Nucleus Scattering Measurements at the SNS

    NASA Astrophysics Data System (ADS)

    Markoff, Diane; Coherent Collaboration

    2015-10-01

    The COHERENT collaboration has proposed to measure coherent, elastic neutrino-nucleus scattering (CE νNS) cross sections on several nuclear targets using neutrinos produced at the Spallation Neutron Source (SNS) located at the Oak Ridge National Laboratory. The largest background of concern arises from beam-induced, fast neutrons that can mimic a nuclear recoil signal event in the detector. Multiple technologies of neutron detection have been employed at prospective experiment sites at the SNS. Analysis of these data have produced a consistent picture of the backgrounds expected for a CE νNS measurement. These background studies show that at suitable locations, the fast neutrons of concern arrive mainly in the prompt 1.3 μs window and the neutrons in the delayed window are primarily of lower energies that are relatively easier to shield.

  6. Neutron-induced charged-particle emission studies below 100 MeV at WNR

    SciTech Connect

    Haight, R.C.; Lee, T.M.; Sterbenz, S.M.

    1994-07-01

    Charged-particles produced by neutron bombardment of selected targets with Z=5 through 53 have been studied for neutron energies from 1 MeV to about 100 MeV using the spallation neutron source at WNR/LAMPF. Particle detection with energy measurement and particle identification is accomplished by two-element {Delta}E-E counters, three-element {Delta}E{sub l}-{Delta}E{sub 2}-E counters or with pulse-shape discrimination using scintillators directly in the neutron beam. The experimental techniques for these measurements are described and comparisons made among the different approaches. This presentation introduces five papers contributed to this conference.

  7. Neutron-induced reactions relevant for Inertial-Cofinement Fusion Experiments

    NASA Astrophysics Data System (ADS)

    Boswell, Melissa; Devlin, Mathew; Fotiadis, Nikolaos; Merrill, Frank; Nelson, Ronald; Tonchev, Anton

    2014-09-01

    The typical ignition experiment at the National Ignition Facility ablatively implodes a plastic capsule filled with DT fuel, generating a high flux of 14-MeV neutrons from the d(t,n) α reaction. There is some spread in the energy of these primary 14-MeV neutrons, which is mainly attributable to Doppler shifting from the relative thermal motion of the burning DT fuel. Neutrons created during this reaction have 5--10% chance of scattering before escaping the fuel assembly, losing some fraction of their energy in the scattering process. Neutrons emerging with an energy greater than the reaction energy are generated by a two-step process where neutrons first transfer momentum to a deuteron or tritium ion, these enhanced energy ions then fuse in flight to produce higher energy neutrons; some of these neutrons have energies in excess of 30 MeV. Measuring the fluencies of both the low- and high-energy neutrons is a powerful mechanism for studying the properties of the fuel assembly, and the various parameters important to inertial confinement fusion. We have developed a number of tools to measure the spectral characteristics of the NIF neutron spectrum. Most of these methods rely on exploiting the energy dependence of (n, γ), (n,2n), (n,3n) and (n,p) reactions on a variety o.

  8. Prompt gamma-ray analysis of chlorine in superpozz cement concrete

    NASA Astrophysics Data System (ADS)

    Naqvi, A. A.; Kalakada, Zameer; Al-Matouq, Faris A.; Maslehuddin, M.; Al-Amoudi, O. S. B.; ur-Rehman, Khateeb

    2012-11-01

    The chlorine concentration in Superpozz (SPZ) cement concrete was analyzed using a newly designed prompt gamma-ray neutron activation (PGNAA) setup utilizing a portable neutron generator. The setup, which mainly consists of a neutron source along with its moderator placed side by side with a shielded gamma-ray detector, allows determining chloride concentration in a concrete structure from one side. The setup has been tested through chlorine detection in chloride-contaminated Superpozz (SPZ) cement concrete specimens using 6.11 and 2.86±3.10 MeV chlorine prompt gamma-rays. The optimum 0.032±0.012 wt% value of Minimum Detectable Concentration (MDC) of chlorine in SPZ cement concrete measured in this study shows a successful application of a portable neutron generator in chloride analysis of concrete structure for corrosion studies.

  9. Relativistic mass ejecta from phase-transition-induced collapse of neutron stars

    SciTech Connect

    Cheng, K.S.; Harko, T.; Tian, X.L.; Huang, Y.F.; Lin, L.M.; Suen, W.M. E-mail: harko@hkucc.hku.hk E-mail: lmlin@phy.cuhk.edu.hk E-mail: tianxiaolei@gmail.com

    2009-09-01

    We study the dynamical evolution of a phase-transition-induced collapse neutron star to a hybrid star, which consists of a mixture of hadronic matter and strange quark matter. The collapse is triggered by a sudden change of equation of state, which result in a large amplitude stellar oscillation. The evolution of the system is simulated by using a 3D Newtonian hydrodynamic code with a high resolution shock capture scheme. We find that both the temperature and the density at the neutrinosphere are oscillating with acoustic frequency. However, they are nearly 180° out of phase. Consequently, extremely intense, pulsating neutrino/antineutrino fluxes will be emitted periodically. Since the energy and density of neutrinos at the peaks of the pulsating fluxes are much higher than the non-oscillating case, the electron/positron pair creation rate can be enhanced dramatically. Some mass layers on the stellar surface can be ejected by absorbing energy of neutrinos and pairs. These mass ejecta can be further accelerated to relativistic speeds by absorbing electron/positron pairs, created by the neutrino and antineutrino annihilation outside the stellar surface. The possible connection between this process and the cosmological Gamma-ray Bursts is discussed.

  10. Heat-induced structural transitions of alpha-crystallin studied by small-angle neutron scattering

    NASA Astrophysics Data System (ADS)

    Krivandin, A. V.; Kuklin, A. I.; Muranov, K. O.; Murugova, T. N.; Kozlov, S. S.; Genkina, N. K.

    2012-03-01

    Alpha-crystallin from the bovine eye lens was studied by small-angle neutron scattering (SANS) in 90% D2O buffer solution at 20, 50, 60, 65, 75, 85 and 95°C. The temperature points for this study were specified on the basis of differential scanning calorimetric analysis of alpha-crystallin solutions which has shown two endothermic transitions with midpoints at 64.5 and 86°C. The SANS study revealed no significant alpha-crystallin quaternary structure alterations at 50°C as compared with 20°C. At 60-65°C the SANS data confirmed substantial alpha-crystallin quaternary structure rearrangements which resulted in the formation of alpha-crystallin oligomers with a similar shape but approximately twofold increased molecular weight as compared to the native state at 20°C. At higher temperatures (75, 85 and 95°C) the SANS patterns were very similar and were consistent with the scattering by rod-like particles with a cross-section radius of gyration ~55 This transformation of alpha-crystallin to the rod-like particles was evidently irreversible as these particles remained in solution after cooling to 20°C. Ab initio shape models of the native and high-temperature alpha-crystallin were retrieved with DAMMIN and DAMAVER software. Schematic model of alpha-crystallin heat-induced quaternary structure transitions was considered.

  11. Bayesian Evaluation Including Covariance Matrices of Neutron-induced Reaction Cross Sections of {sup 181}Ta

    SciTech Connect

    Leeb, H. Schnabel, G.; Srdinko, Th.; Wildpaner, V.

    2015-01-15

    A new evaluation of neutron-induced reactions on {sup 181}Ta using a consistent procedure based on Bayesian statistics is presented. Starting point of the evaluation is the description of nuclear reactions via nuclear models implemented in TALYS 1.4. A retrieval of experimental data was performed and covariance matrices of the experiments were generated from an extensive study of the corresponding literature. All reaction channels required for a transport file up to 200 MeV have been considered and the covariance matrices of cross section uncertainties for the most important channels are determined. The evaluation has been performed in one step including all available experimental data. A comparison of the evaluated cross sections and spectra with experimental data and available evaluations is performed. In general the evaluated cross section reflect our best knowledge and give a fair description of the observables. However, there are few deviations from expectation which clearly indicate the impact of the prior and the need to account for model defects. Using the results of the evaluation a complete ENDF-file similarly to those of the TENDL library is generated.

  12. Analysis of Induced Gamma Activation by D-T Neutrons in Selected Fusion Reactor Relevant Materials with EAF-2010

    NASA Astrophysics Data System (ADS)

    Klix, Axel; Fischer, Ulrich; Gehre, Daniel

    2016-02-01

    Samples of lanthanum, erbium and titanium which are constituents of structural materials, insulating coatings and tritium breeder for blankets of fusion reactor designs have been irradiated in a fusion peak neutron field. The induced gamma activities were measured and the results were used to check calculations with the European activation system EASY-2010. Good agreement for the prediction of major contributors to the contact dose rate of the materials was found, but for minor contributors the calculation deviated up to 50%.

  13. Application of an in vivo mutagenesis system to assess aminothiol effects on neutron-induced genotoxic damage in mouse spleenocytes

    SciTech Connect

    Basic, I. . Dept. of Animal Physiology); Grdina, D.J.; Lyons, T. )

    1989-01-01

    A cloning technique has been developed to quantitate and study {ital in vivo} somatic mutations at the hypoxanthine-guanine phosphoribosyl transferase (HGPRT) locus in human lymphocytes. In this paper we describe a modification of this assay to quantify HGPRT mutations in mouse spleenocytes. In particular, we have investigated the effects of the aminothiol on mutagenesis induced by single doses of whole body exposures to fission-spectrum neutrons from the JANUS reactor at Argonne National Laboratory. 7 refs., 3 tabs.

  14. Cosmic-ray-induced neutron intensity in Taiwan and its variations during a typhoon

    NASA Astrophysics Data System (ADS)

    Chung, C.; Chen, C. Y.

    Cosmic neutrons, as a secondary cosmic radiation, strike the ground with intensity which varies at different latitude, altitude, and solar activity. In a 3-year extensive survey period, the cosmic neutron intensity was measured over Taiwan islandwide; the average neutron dose equivalent rate is 0.65nSvh-1 near sea level, up to 14.5nSvh-1 at the highest mountaintop (altitude of 3952 m). In a rare event, the cosmic neutron intensity at a monitoring station was recorded during the entire period that Typhoon Herb swept across the island in 1996. The anomalous reading of cosmic neutron intensity in the typhoon eye, 2.17+/-0.40nSvh-1 (or 4 times higher than the normal reading) is reported here for the first time. The onset of cosmic neutron intensity in the typhoon is closely associated with the steady, rapid air pressure drop as well as the 6×106km3 spiral cloud; the dips in the onset are correlated with sustained gale winds and heavy precipitation. It is believed that the air pressure drop provides thinner air within the typhoon, and the spiral cloud containing dense moisture further slows down high energy neutrons from the ground, where we observed the neutrons showering down from the stratosphere where the cosmic neutrons have the maximum density. These combined effects result in more medium-energy neutrons penetrating down to the ground through the typhoon; while the gale wind and heavy rain deflect, attenuate, and, to a lesser extent, absorb the cosmic neutrons from the atmosphere.

  15. Neutron-Induced Fission Cross Sections of Nuclei in the Vicinity of 208Pb at Incident Energies below 60 MeV

    NASA Astrophysics Data System (ADS)

    Ryzhov, Igor V.; Tutin, Gennady A.; Eismont, Vilen P.; Mitryukhin, Andrey G.; Oplavin, Valery S.; Soloviev, Sergey M.; Meulders, Jean-Pierre; El Masri, Youssef; Keutgen, Thomas; Prieels, René; Nolte, Ralf

    2005-05-01

    Neutron-induced fission cross sections of 205Tl, 204, 206, 207, 208Pb, and 209Bi have been measured at incident energies of 32.8, 45.3, and 59.9 MeV. The measurements were performed at the Louvain-la-Neuve neutron beam facility using the 7Li (p, n) reaction as neutron source. Fission fragments were detected with a multi-section Frisch-gridded ionization chamber (MFGIC). Neutron fluence measurements were based on the 238U(n, f) reaction. The neutron fluence monitoring procedure was asserted by crosscheck measurement, in which the 59.9-MeV neutron beam fluence was simultaneously determined with the MFGIC and with a fission chamber monitor calibrated relative to a proton-recoil telescope.

  16. Neutron fluence rate measurements in a PGNAA 208-liter drum assay system using silicon carbide detectors

    NASA Astrophysics Data System (ADS)

    Dulloo, A. R.; Ruddy, F. H.; Seidel, J. G.; Lee, S.; Petrović, B.; McIlwain, M. E.

    2004-01-01

    Pulsed prompt gamma neutron activation analysis (PGNAA) is being implemented for the nondestructive assay (NDA) of mercury, cadmium and lead in containers of radioactive waste. A PGNAA prototype system capable of assaying 208-liter (55-gallon) drums has already been built and demonstrated. As part of the evaluation of this system, the thermal neutron fluence rate distribution in a drum containing a combustible waste surrogate was measured during PGNAA runs using a silicon carbide neutron detector. The fast charge-collection time of this detector type enabled the investigation of the neutron kinetics at various locations within the matrix during and between pulses of the system's 14-MeV neutron source. As expected, the response of a SiC detector equipped with a lithium-6 fluoride layer is dominated by thermal neutron-induced events between pulses. The measurement results showed that the thermal neutron fluence rate is relatively uniform over a radial depth of several centimeters in the matrix region that contributes a significant fraction of the prompt gamma radiation incident on the system's photon detector.

  17. Measurement of Fragment Mass Yields in Neutron-Induced Fission of 232TH and 238U at 33, 45 and 60 Mev

    NASA Astrophysics Data System (ADS)

    Simutkin, V. D.; Pomp, S.; Blomgren, J.; Österlund, M.; Andersson, P.; Bevilacqua, R.; Ryzhov, I. V.; Tutin, G. A.; Khlopin, V. G.; Onegin, M. S.; Vaishnene, L. A.; Meulders, J. P.; Prieels, R.

    2011-10-01

    Over the past years, a significant effort has been devoted to measurements of neutron-induced fission cross-sections at intermediate energies but there is a lack of experimental data on fission yields. Here we describe recent measurements of pre-neutron emission fragment mass distributions from intermediate energy neutron-induced fission of 232Th and 238U. The measurements have been done at the quasi-monoenergetic neutron beam of the Louvain-la-Neuve cyclotron facility CYCLONE and neutron peak energies at 32.8, 45.3 and 59.9 MeV. A multi-section Frisch-gridded ionization chamber was used as a fission fragment detector. The measurement results are compared with available experimental data. Some TALYS code modifications done to describe the experimental results are discussed.

  18. Stress-induced martensitic transformations in NiTi and NiTi-TiC composites investigated by neutron diffraction

    SciTech Connect

    Vaidyanathan, R.; Bourke, M.A.M.; Dunand, D.C.

    1998-12-31

    Superelastic NiTi (51.0 at% Ni) with 0, 10 and 20 vol% TiC particles were deformed under uniaxial compression as neutron diffraction spectra were simultaneously obtained. The experiments yielded in-situ measurements of the thermoelastic stress-induced transformation. A detailed Rietveld determination is made of the phase fractions and the evolving strains in the reinforcing TiC particles and the austenite as it transforms to martensite on loading (and its subsequent back transformation on unloading). These strains are used to shed light on the phenomenon of load transfer in composites where the matrix undergoes a stress-induced phase transformation.

  19. Neutron yield enhancement in laser-induced deuterium-deuterium fusion using a novel shaped target.

    PubMed

    Zhao, J R; Zhang, X P; Yuan, D W; Chen, L M; Li, Y T; Fu, C B; Rhee, Y J; Li, F; Zhu, B J; Li, Yan F; Liao, G Q; Zhang, K; Han, B; Liu, C; Huang, K; Ma, Y; Li, Yi F; Xiong, J; Huang, X G; Fu, S Z; Zhu, J Q; Zhao, G; Zhang, J

    2015-06-01

    Neutron yields have direct correlation with the energy of incident deuterons in experiments of laser deuterated target interaction [Roth et al., Phys. Rev. Lett. 110, 044802 (2013) and Higginson et al., Phys. Plasmas 18, 100703 (2011)], while deuterated plasma density is also an important parameter. Experiments at the Shenguang II laser facility have produced neutrons with energy of 2.45 MeV using d (d, n) He reaction. Deuterated foil target and K-shaped target were employed to study the influence of plasma density on neutron yields. Neutron yield generated by K-shaped target (nearly 10(6)) was two times higher than by foil target because the K-shaped target results in higher density plasma. Interferometry and multi hydro-dynamics simulation confirmed the importance of plasma density for enhancement of neutron yields. PMID:26133837

  20. Neutron yield enhancement in laser-induced deuterium-deuterium fusion using a novel shaped target

    SciTech Connect

    Zhao, J. R.; Chen, L. M. Li, Y. T.; Li, F.; Zhu, B. J.; Li, Yan. F.; Liao, G. Q.; Huang, K.; Ma, Y.; Li, Yi. F.; Zhang, X. P.; Fu, C. B.; Yuan, D. W.; Zhang, K.; Han, B.; Zhao, G.; Rhee, Y. J.; Liu, C.; Xiong, J.; Huang, X. G.; and others

    2015-06-15

    Neutron yields have direct correlation with the energy of incident deuterons in experiments of laser deuterated target interaction [Roth et al., Phys. Rev. Lett. 110, 044802 (2013) and Higginson et al., Phys. Plasmas 18, 100703 (2011)], while deuterated plasma density is also an important parameter. Experiments at the Shenguang II laser facility have produced neutrons with energy of 2.45 MeV using d (d, n) He reaction. Deuterated foil target and K-shaped target were employed to study the influence of plasma density on neutron yields. Neutron yield generated by K-shaped target (nearly 10{sup 6}) was two times higher than by foil target because the K-shaped target results in higher density plasma. Interferometry and multi hydro-dynamics simulation confirmed the importance of plasma density for enhancement of neutron yields.

  1. Initial observations of cavitation-induced erosion of liquid metal spallation target vessels at the Spallation Neutron Source

    NASA Astrophysics Data System (ADS)

    McClintock, D. A.; Riemer, B. W.; Ferguson, P. D.; Carroll, A. J.; Dayton, M. J.

    2012-12-01

    During operation of the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory the mechanical properties of the AISI 316L target module are altered by high-energy neutron and proton radiation. The interior surfaces of the target vessel are also damaged by cavitation-induced erosion, which results from repetitive rapid heating of the liquid mercury by high-energy proton beam pulses. Until recently no observations of cavitation-induced erosion were possible for conditions fully prototypic to the SNS. Post-Irradiation Examination (PIE) of the first and second operational SNS targets was performed to gain insight into the radiation-induced changes in mechanical properties of the 316L target material and the extent of cavitation-induced erosion to the mercury vessel inner surfaces. Observations of cavitation-induced erosion of the first and second operational SNS target modules are presented here, including images of the target vessel interiors and specimens removed from the target beam-entrance regions.

  2. Neutron induced fission of 238U at incident neutron energies from 1.2 to 5.8 MeV

    NASA Astrophysics Data System (ADS)

    Vivès, F.; Hambsch, F.-J.; Oberstedt, S.; Barreau, G.; Bax, H.

    1998-10-01

    The reaction 238U(n,f) has been studied at IRMM at different incident neutron energies ranging from En=1.2 to 5.8 MeV. The existence of vibrational resonances in the region of the threshold of the fission cross-section and the proton pairing effect should induce variations in the fission fragment properties. The fission fragment mass, mean total kinetic energy (TKE¯) and angular distributions have been investigated with a double Frisch-gridded ionization chamber. For each incident neutron energy, more than 105 events have been accumulated. The TKE¯ shows an increasing trend up to En=3.5 MeV with a sudden drop at roughly En=3.8 MeV which might be related to the onset of pair breaking. Above En=3.8 MeV TKE¯ is again continually increasing. The two-dimensional mass-TKE distributions have been compared by means of a fit with theoretical calculations performed recently in the frame of the multi-modal random neck-rupture model. Actually, two solutions are possible with assuming either two or three Gaussians for the asymmetric part of the mass distribution. However, both solutions lead to the same physical interpretation. The solution with three Gaussians is more in line with the theoretical predictions. In any case the super-long symmetric mode has to be included, in order to explain the dip in TKE¯ close to symmetry.

  3. Application of the Trojan Horse Method to study neutron induced reactions: the 17O(n, α)14C reaction

    NASA Astrophysics Data System (ADS)

    Gulino, M.; Spitaleri, C.; Tang, X. D.; Guardo, G. L.; Lamia, L.; Cherubini, S.; Bucher, B.; Burjan, V.; Couder, M.; Davies, P.; deBoer, R.; Fang, X.; Goldberg, V. Z.; Hons, Z.; Kroha, V.; Lamm, L.; La Cognata, M.; Li, C.; Ma, C.; Mrazek, J.; Mukhamedzhanov, A. M.; Notani, M.; O'Brien, S.; Pizzone, R. G.; Rapisarda, G. G.; Roberson, D.; Sergi, M. L.; Tan, W.; Thompson, I. J.; Wiescher, M.

    2014-03-01

    The reaction 17O(n, α)14C was studied using virtual neutrons coming from the quasi-free deuteron break-up in the three body reaction 17O+d → α+14C+p. This technique, called virtual neutron method, extends the Trojan Horse method to neutron-induced reactions allowing to study the reaction cross section avoiding the suppression effects coming from the penetrability of the centrifugal barrier. For incident neutron energies from thermal up to a few hundred keV, direct experiments have shown the population of two out of three expected excited states at energies 8213 keV and 8282 keV and the influence of the sub-threshold level at 8038 keV. In the present experiment the 18O excited state at E* = 8.125 MeV, missing in the direct measurement, is observed. The angular distributions of the populated resonances have been measured for the first time. The results unambiguously indicate the ability of the method to overcome the centrifugal barrier suppression effect and to pick out the contribution of the bare nuclear interaction.

  4. Neutron-induced electronic failures around a high-energy linear accelerator

    SciTech Connect

    Kry, Stephen F.; Johnson, Jennifer L.; White, R. Allen; Howell, Rebecca M.; Kudchadker, Rajat J.; Gillin, Michael T.

    2011-01-15

    Purpose: After a new in-vault CT-on-rails system repeatedly malfunctioned following use of a high-energy radiotherapy beam, we investigated the presence and impact of neutron radiation on this electronic system, as well as neutron shielding options. Methods: We first determined the CT scanner's failure rate as a function of the number of 18 MV monitor units (MUs) delivered. We then re-examined the failure rate with both 2.7-cm-thick and 7.6-cm-thick borated polyethylene (BPE) covering the linac head for neutron shielding. To further examine shielding options, as well as to explore which neutrons were relevant to the scanner failure, Monte Carlo simulations were used to calculate the neutron fluence and spectrum in the bore of the CT scanner. Simulations included BPE covering the CT scanner itself as well as covering the linac head. Results: We found that the CT scanner had a 57% chance of failure after the delivery of 200 MUs. While the addition of neutron shielding to the accelerator head reduced this risk of failure, the benefit was minimal and even 7.6 cm of BPE was still associated with a 29% chance of failure after the delivery of 200 MU. This shielding benefit was achieved regardless of whether the linac head or CT scanner was shielded. Additionally, it was determined that fast neutrons were primarily responsible for the electronic failures. Conclusions: As illustrated by the CT-on-rails system in the current study, physicists should be aware that electronic systems may be highly sensitive to neutron radiation. Medical physicists should therefore monitor electronic systems that have not been evaluated for potential neutron sensitivity. This is particularly relevant as electronics are increasingly common in the therapy vault and newer electronic systems may exhibit increased sensitivity.

  5. Smectic order induced at homeotropically aligned nematic surfaces: a neutron reflection study.

    PubMed

    Lau, Y G J; Richardson, Robert M; Cubitt, R

    2006-06-21

    Neutron reflection was used to measure the buildup of layers at a solid surface as the smectic phase is approached from higher temperatures in a nematic liquid crystal. The liquid crystal was 4-octyl-4'-cyanobiphenyl (8CB), and the solid was silicon with one of five different surface treatments that induce homeotropic alignment: (i) silicon oxide; (ii) a cetyltrimethylammonium bromide coating; (iii) an octadecyltrichlorosilane monolayer; (iv) an n-n-dimethyl-n-octadecyl-3- aminopropyltrimethyloxysilyl chloride monolayer; and (v) a lecithin coating. The development of surface smectic layers in the nematic phase of 8CB was followed by measuring specular reflectivity and monitoring the pseudo-Bragg peak from the layers. The scattering data were processed to remove the scattering from short-ranged smecticlike fluctuations in the bulk nematic phase from the specular reflection. The pseudo-Bragg peak at scattering vector Q approximately 0.2 A(-1) therefore corresponded to the formation of long-range smectic layers at the surface. The amplitude of the smectic density wave decayed with increasing distance from the surface, and the characteristic thickness of this smectic region diverged as the transition temperature was approached. It was found that the characteristic thickness for some of the surface treatments was greater than the correlation length in the bulk nematic. The different surfaces gave different values of the smectic order parameter at the surface. This suggests that the interaction with the surface is significantly different from a "hard wall" which would give the same values of the smectic order parameter and penetration depths similar to the bulk correlation length. Comparison of the different surfaces also suggested that the strength and range of the surface smectic ordering may be varied independently. PMID:16821956

  6. Production, Distribution, and Applications of Californium-252 Neutron Sources

    SciTech Connect

    Balo, P.A.; Knauer, J.B.; Martin, R.C.

    1999-10-03

    The radioisotope {sup 252}Cf is routinely encapsulated into compact, portable, intense neutron sources with a 2.6-year half-life. A source the size of a person's little finger can emit up to 10{sup 11} neutrons/s. Californium-252 is used commercially as a reliable, cost-effective neutron source for prompt gamma neutron activation analysis (PGNAA) of coal, cement, and minerals, as well as for detection and identification of explosives, laud mines, and unexploded military ordnance. Other uses are neutron radiography, nuclear waste assays, reactor start-up sources, calibration standards, and cancer therapy. The inherent safety of source encapsulations is demonstrated by 30 years of experience and by U.S. Bureau of Mines tests of source survivability during explosions. The production and distribution center for the U. S Department of Energy (DOE) Californium Program is the Radiochemical Engineering Development Center (REDC) at Oak Ridge National Laboratory (ORNL). DOE sells The radioisotope {sup 252}Cf is routinely encapsulated into compact, portable, intense neutron sources with a 2.6- year half-life. A source the size of a person's little finger can emit up to 10 neutrons/s. Californium-252 is used commercially as a reliable, cost-effective neutron source for prompt gamma neutron activation analysis (PGNAA) of coal, cement, and minerals, as well as for detection and identification of explosives, laud mines, and unexploded military ordnance. Other uses are neutron radiography, nuclear waste assays, reactor start-up sources, calibration standards, and cancer therapy. The inherent safety of source encapsulations is demonstrated by 30 years of experience and by U.S. Bureau of Mines tests of source survivability during explosions. The production and distribution center for the U. S Department of Energy (DOE) Californium Program is the Radiochemical Engineering Development Center (REDC) at Oak Ridge National Laboratory(ORNL). DOE sells {sup 252}Cf to commercial

  7. Evaluation of (α,n) induced neutrons as a background for dark matter experiments

    NASA Astrophysics Data System (ADS)

    Mei, D.-M.; Zhang, C.; Hime, A.

    2009-07-01

    Neutrons from (α,n) reactions through thorium and uranium decays are important sources of background for direct dark matter detection. The neutron yields and energy spectra from a range of materials that are used to build dark matter detectors are calculated and tabulated. In addition to thorium and uranium decays, we found that α-particles from samarium, often the dopant of the window materials of photomultiplier tubes (PMT), are also an important source of neutron yield. The results in this paper can be used as the input to Monte Carlo simulations for many materials that will be used for next generation experiments.

  8. Long-range electrostatics-induced two-proton transfer captured by neutron crystallography in an enzyme catalytic site

    DOE PAGESBeta

    Gerlits, Oksana; Wymore, Troy; Das, Amit; Shen, Chen -Hsiang; Parks, Jerry M.; Smith, Jeremy C.; Weiss, Kevin L.; Keen, David A.; Blakeley, Matthew P.; Louis, John M.; et al

    2016-03-09

    Neutron crystallography was used to directly locate two protons before and after a pH-induced two-proton transfer between catalytic aspartic acid residues and the hydroxy group of the bound clinical drug darunavir, located in the catalytic site of enzyme HIV-1 protease. The two-proton transfer is triggered by electrostatic effects arising from protonation state changes of surface residues far from the active site. The mechanism and pH effect are supported by quantum mechanics/molecular mechanics (QM/MM) calculations. The low-pH proton configuration in the catalytic site is deemed critical for the catalytic action of this enzyme and may apply more generally to other asparticmore » proteases. Neutrons therefore represent a superb probe to obtain structural details for proton transfer reactions in biological systems at a truly atomic level.« less

  9. Investigation of the maximum accessible kinetic energy of fragments in the neutron-induced fission of {sup 238}U nuclei

    SciTech Connect

    Khryachkov, V. A. Bondarenko, I. P.; Ivanova, T. A.; Kuzminov, B. D.; Semenova, N. N.; Sergachev, A. I.

    2013-03-15

    The masses, total kinetic energies (TKE), and emission angles of fragments originating from the fission of {sup 238}U nuclei that was induced by 5- and 6.5-MeV neutrons were measured by using digital methods for processing signals. A detailed analysis of the shape of digital signals made it possible to reduce substantially the contribution of fragments whose TKE values were distorted because of a superimposition of signals from recoil protons and from alpha particles produced in the spontaneous decay of uranium. The total statistics exceeded two million events for either neutron energy, and this permitted performing a detailed analysis of fission-fragment yields in the region of the highest attainable TKE values. An analysis of fragment yields made it possible to draw specific conclusions on the structure of the potential surface of fissile nuclei.

  10. Cross Sections for Neutron-induced Reactions on Actinide Targets Extracted from Surrogate Experiments: A Status Report

    SciTech Connect

    Escher, J E; Burke, J T; Dietrich, F S; Lesher, S R; Scielzo, N D; Thompson, I J; Younes, W

    2009-10-01

    The Surrogate nuclear reactions method, an indirect approach for determining cross sections for compound-nuclear reactions involving difficult-to-measure targets, is reviewed. Focusing on cross sections for neutron-induced reactions on actinides, we review the successes of past and present applications of the method and assess its uncertainties and limitations. The approximations used in the analyses of most experiments work reasonably well for (n,f) cross sections for neutron energies above 1-2 MeV, but lead to discrepancies for low-energy (n,f) reactions, as well as for (n,{gamma}) applications. Correcting for some of the effects neglected in the approximate analyses leads to improved (n,f) results. We outline steps that will further improve the accuracy and reliability of the Surrogate method and extend its applicability to reactions that cannot be approached with the present implementation of the method.

  11. Long-Range Electrostatics-Induced Two-Proton Transfer Captured by Neutron Crystallography in an Enzyme Catalytic Site.

    PubMed

    Gerlits, Oksana; Wymore, Troy; Das, Amit; Shen, Chen-Hsiang; Parks, Jerry M; Smith, Jeremy C; Weiss, Kevin L; Keen, David A; Blakeley, Matthew P; Louis, John M; Langan, Paul; Weber, Irene T; Kovalevsky, Andrey

    2016-04-11

    Neutron crystallography was used to directly locate two protons before and after a pH-induced two-proton transfer between catalytic aspartic acid residues and the hydroxy group of the bound clinical drug darunavir, located in the catalytic site of enzyme HIV-1 protease. The two-proton transfer is triggered by electrostatic effects arising from protonation state changes of surface residues far from the active site. The mechanism and pH effect are supported by quantum mechanics/molecular mechanics (QM/MM) calculations. The low-pH proton configuration in the catalytic site is deemed critical for the catalytic action of this enzyme and may apply more generally to other aspartic proteases. Neutrons therefore represent a superb probe to obtain structural details for proton transfer reactions in biological systems at a truly atomic level. PMID:26958828

  12. Measurement of the muon-induced neutron yield in liquid scintillator and stainless steel at LNGS with the LVD experiment

    SciTech Connect

    Persiani, R.; Garbini, M.; Sartorelli, G.; Selvi, M.; Collaboration: LVD Collaboration

    2013-08-08

    We describe the measurement of the muon-induced neutron yield in liquid scintillator and stainless steel (SS) at the Gran Sasso National Laboratory (LNGS), with the LVD experiment. The Large Volume Detector (LVD) is located in Hall A of the LNGS and is made of 1000 t of liquid scintillator and 1000 t of SS. Using an independent measurement to evaluate the background and with the support of a full Monte Carlo simulation based on Geant4, we measured a neutron yield of (2.9±0.6)×10{sup −4} and (1.5±0.3)×10{sup −3} in liquid scintillator and in stainless steel, respectively.

  13. Experimental and simulation studies of neutron-induced single-event burnout in SiC power diodes

    NASA Astrophysics Data System (ADS)

    Shoji, Tomoyuki; Nishida, Shuichi; Hamada, Kimimori; Tadano, Hiroshi

    2014-01-01

    Neutron-induced single-event burnouts (SEBs) of silicon carbide (SiC) power diodes have been investigated by white neutron irradiation experiments and transient device simulations. It was confirmed that a rapid increase in lattice temperature leads to formation of crown-shaped aluminum and cracks inside the device owing to expansion stress when the maximum lattice temperature reaches the sublimation temperature. SEB device simulation indicated that the peak lattice temperature is located in the vicinity of the n-/n+ interface and anode contact, and that the positions correspond to a hammock-like electric field distribution caused by the space charge effect. Moreover, the locations of the simulated peak lattice temperature agree closely with the positions of the observed destruction traces. Furthermore, it was theoretically demonstrated that the period of temperature increase of a SiC power device is two orders of magnitude less than that of a Si power device, using a thermal diffusion equation.

  14. Calculated neutron-induced cross sections for /sup 53/Cr from 1 to 20 MeV

    SciTech Connect

    Shibata, K.; Hetrick, D.M.

    1987-05-01

    Neutron-induced cross sections of /sup 53/Cr have been calculated in the energy regions from 1 to 20 MeV. The quantities obtained are the cross sections for the reactions (n,n'..gamma..), (n,2n), (n,np), (n,n..cap alpha..), (n,p..gamma..), (n,pn), (n,..cap alpha gamma..), (n,..cap alpha..n), (n,d), (n,t), (n,/sup 3/He), and (n,..gamma..), as well as the spectra of emitted neutrons, protons, alpha particles, and gamma rays. The precompound process was included above 5 MeV in addition to the compound process. For the inelastic scattering, the contribution of the direct interaction was calculated with DWBA. 36 refs., 23 figs., 11 tabs.

  15. Evaluation of {sup 28,29,30}Si neutron induced cross sections for ENDF/B-VI

    SciTech Connect

    Hetrick, D.M.; Larson, D.C.; Larson, N.M.; Leal, L.C.; Epperson, S.J.

    1997-04-01

    Separate evaluations have been done for the three stable isotopes of silicon for ENDF/B-VI. The evaluations are based on analysis of experimental data, supplemented by results of nuclear model calculations. The computational methods and the parameters required as input to the nuclear model codes are reviewed. Discussion of the evaluated data given for resonance parameters, neutron induced reaction cross sections, associated angular and energy distributions, and gamma-ray production cross sections is included. Extensive comparisons of the evaluated cross sections to measured data are shown in this report. The evaluations include all necessary data to allow KERMA (Kinetic Energy Released in MAterials) and displacement cross sections to be calculated directly. These quantities are fundamental to studies of neutron heating and radiation damage.

  16. Combined neutron imaging techniques for cultural heritage purpose

    SciTech Connect

    Materna, T.

    2009-01-28

    This article presents the different new neutron techniques developed by the Ancient Charm collaboration to image objects of cultural heritage importance: Prompt-gamma-ray activation imaging (PGAI) coupled to cold/thermal neutron transmission tomography, Neutron Resonance Capture Imaging (NRCI) and Neutron Resonance Tomography.

  17. Neutron-Induced Reactions on Copper and Zero-Neutrino Double-Beta Decay Searches

    NASA Astrophysics Data System (ADS)

    Gooden, Matthew; Kelley, John; Fallin, Brent; Finch, Sean; Howell, Calvin; Rusev, Gencho; Tonchev, Anton; Tornow, Werner

    2012-10-01

    Cross-section measurements of (n,xγ) reactions on ^natCu were carried out at TUNL using monoenergetic neutrons at six energies of En = 6, 8, 10, 12, 14, 16 MeV. These studies were performed to provide accurate cross-section data on materials abundant in experimental setups involving HPGe detectors used to search for rare events, like the neutrino-less double-beta decay of ^76Ge. Spallation and (α,n) neutrons are expected to cause the largest source of external background in the energy region of interest. At TUNL pulsed neutron beams were produced via the ^2H(d,n)^3He reaction and the deexcitation γ rays from the reaction ^natCu(n,xγ) were detected with clover HPGe detectors. Our cross-section data will be compared to theoretical calculations and to data recently obtained at LANL with a white neutron beam.

  18. Borehole parametric study for neutron induced capture gamma-ray spectrometry using the MCNP code.

    PubMed

    Shahriari, M; Sohrabpour, M

    2000-01-01

    The MCNP Monte Carlo code has been used to simulate neutron transport from an Am-Be source into a granite formation surrounding a borehole. The effects of the moisture and the neutron poison on the thermal neutron flux distribution and the capture by the absorbing elements has been calculated. Thermal and nonthermal captures for certain absorbers having resonance structures in the epithermal and fast energy regions such as W and Si were performed. It is shown that for those absorbers having large resonances in the epithermal regions when they are present in dry formation or when accompanied by neutron poisons the resonance captures may be significant compared to the thermal captures. PMID:10670932

  19. 45 CFR 1701.5 - Prompt response.

    Code of Federal Regulations, 2011 CFR

    2011-10-01

    ... 45 Public Welfare 4 2011-10-01 2011-10-01 false Prompt response. 1701.5 Section 1701.5 Public Welfare Regulations Relating to Public Welfare (Continued) NATIONAL COMMISSION ON LIBRARIES AND INFORMATION SCIENCE DISCLOSURE OF INFORMATION § 1701.5 Prompt response. (a) Within ten days...

  20. Song Prompts: I Had a Cat

    ERIC Educational Resources Information Center

    Kenney, Susan Hobson

    2011-01-01

    This article discusses song prompts as a way to encourage children to sing during exploratory play. A song prompt for "I Had a Cat" is included for educators to try in their own classrooms or preschools. Educators are invited to share ideas they have used that encourage children to sing during free play.

  1. Say Cheese! Using Personal Photographs as Prompts.

    ERIC Educational Resources Information Center

    Lazarus, Belinda Davis

    1998-01-01

    Describes the use of photographs showing students engaging in appropriate behavior to prompt students to manage their own classroom behavior more effectively. The article gives examples of appropriate photographs and explains how to teach students to use the prompts. Inserts list photography resources and suggest classroom uses for digital…

  2. 21 CFR 1401.7 - Prompt response.

    Code of Federal Regulations, 2010 CFR

    2010-04-01

    ... 21 Food and Drugs 9 2010-04-01 2010-04-01 false Prompt response. 1401.7 Section 1401.7 Food and Drugs OFFICE OF NATIONAL DRUG CONTROL POLICY PUBLIC AVAILABILITY OF INFORMATION § 1401.7 Prompt response. The General Counsel, or designee, will determine within 20 days (excepting Saturdays, Sundays...

  3. Generalized Instruction following with Pictorial Prompts

    ERIC Educational Resources Information Center

    Phillips, Cara L.; Vollmer, Timothy R.

    2012-01-01

    The benefits of permanent pictorial prompts in enhancing maintenance and generalization are likely dependent on their degree of stimulus control and the extent to which their use is generalized. Although several studies on the use of pictorial prompts have demonstrated their efficacy (e.g., Pierce & Schreibman, 1994; Wacker & Berg, 1983; Wacker,…

  4. 5 CFR 1631.8 - Prompt response.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... Disclosure of Records Under the Freedom of Information Act, 5 U.S.C. 552 § 1631.8 Prompt response. (a)(1... 5 Administrative Personnel 3 2010-01-01 2010-01-01 false Prompt response. 1631.8 Section 1631.8... so advise the requester within 5 work days. The time limit for processing such a request will...

  5. 5 CFR 1631.8 - Prompt response.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... 5 Administrative Personnel 3 2013-01-01 2013-01-01 false Prompt response. 1631.8 Section 1631.8 Administrative Personnel FEDERAL RETIREMENT THRIFT INVESTMENT BOARD AVAILABILITY OF RECORDS Production or Disclosure of Records Under the Freedom of Information Act, 5 U.S.C. 552 § 1631.8 Prompt response....

  6. 5 CFR 1631.8 - Prompt response.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... 5 Administrative Personnel 3 2011-01-01 2011-01-01 false Prompt response. 1631.8 Section 1631.8 Administrative Personnel FEDERAL RETIREMENT THRIFT INVESTMENT BOARD AVAILABILITY OF RECORDS Production or Disclosure of Records Under the Freedom of Information Act, 5 U.S.C. 552 § 1631.8 Prompt response. (a)(1) When the FOIA Officer receives a...

  7. 5 CFR 1631.8 - Prompt response.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... 5 Administrative Personnel 3 2014-01-01 2014-01-01 false Prompt response. 1631.8 Section 1631.8 Administrative Personnel FEDERAL RETIREMENT THRIFT INVESTMENT BOARD AVAILABILITY OF RECORDS Production or Disclosure of Records Under the Freedom of Information Act, 5 U.S.C. 552 § 1631.8 Prompt response....

  8. 5 CFR 1631.8 - Prompt response.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... 5 Administrative Personnel 3 2012-01-01 2012-01-01 false Prompt response. 1631.8 Section 1631.8 Administrative Personnel FEDERAL RETIREMENT THRIFT INVESTMENT BOARD AVAILABILITY OF RECORDS Production or Disclosure of Records Under the Freedom of Information Act, 5 U.S.C. 552 § 1631.8 Prompt response....

  9. 45 CFR 1701.5 - Prompt response.

    Code of Federal Regulations, 2010 CFR

    2010-10-01

    ... 45 Public Welfare 4 2010-10-01 2010-10-01 false Prompt response. 1701.5 Section 1701.5 Public Welfare Regulations Relating to Public Welfare (Continued) NATIONAL COMMISSION ON LIBRARIES AND INFORMATION SCIENCE DISCLOSURE OF INFORMATION § 1701.5 Prompt response. (a) Within ten days...

  10. Identification of neutron irradiation induced strain rate sensitivity change using inverse FEM analysis of Charpy test

    NASA Astrophysics Data System (ADS)

    Haušild, Petr; Materna, Aleš; Kytka, Miloš

    2015-04-01

    A simple methodology how to obtain additional information about the mechanical behaviour of neutron-irradiated WWER 440 reactor pressure vessel steel was developed. Using inverse identification, the instrumented Charpy test data records were compared with the finite element computations in order to estimate the strain rate sensitivity of 15Ch2MFA steel irradiated with different neutron fluences. The results are interpreted in terms of activation volume change.

  11. Fission Fragment Distributions and Delayed Neutron Yields from Photon-Induced-Fission

    SciTech Connect

    David, J.-C.; Dore, D.; Giacri-Mauborgne, M.-L.; Ridikas, D.; Lauwe, A. van

    2005-05-24

    Fission fragment distributions and delayed neutron yields for 235U and 238U are provided by a complete modelization of the photofission process below 25 MeV. The absorption cross-section parameterization and the fission fragment distributions are given and compared to experimental data. The delayed neutron yields and the half-lives in terms of six groups are presented and compared to data obtained with a bremsstrahlung spectrum of 15 MeV.

  12. A new approach for the prediction of the neutron-induced SEU rate

    SciTech Connect

    Vial, C.; Palau, J.M.; Gasiot, J.; Calvet, M.C.; Fourtine, S.

    1998-12-01

    A new approach for SEU rate prediction in components submitted to neutron environment is presented. The method aims to take into account the characteristics of the secondary particles in terms of electrical effect. So, in addition to the critical energy/charge criterion generally used until now, two criteria are tentatively proposed: a critical LET and a limited distance in which energy must be deposited. The starting point of each computation is a common neutron-silicon interaction database.

  13. Resonance Analysis and Evaluation of the Uranium -235 Neutron-Induced Cross-Sections

    NASA Astrophysics Data System (ADS)

    Leal, Luiz Carlos

    Neutron cross sections of fissile nuclei are of considerable interest for the understanding of parameters such as resonance absorption, resonance escape probability, resonance self-shielding, and the dependence of the reactivity on temperature. In the present study, new techniques for the evaluation of the ^{235}U neutron cross sections are described. The Reich-Moore formalism of the Bayesian computer code SAMMY was used to perform consistent R-matrix multilevel analyses of the selected neutron cross-section data. The Delta_3 -statistics of Dyson and Mehta, along with high -resolution data and the spin-separated fission cross-section data, have provided the possibility of developing a new methodology for the analysis and evaluation of neutron -nucleus cross-sections. The result of the analysis consists of a set of resonance parameters which describe the ^{235}U neutron cross sections up to 500 eV. The set of resonance parameters obtained through a R-matrix analysis are expected to satisfy statistical properties which lead to information on the nuclear structure. The resonance parameters were tested and showed good agreement with the theory. It is expected that the parametrization of the ^{235}U neutron cross sections obtained in this dissertation represents the current state of art in data as well as in theory and, therefore, can be of direct use in reactor calculations.

  14. Time features of delayed neutrons and partial emissive-fission cross sections for the neutron-induced fission of {sup 232}Th nuclei in the energy range 3.2-17.9 MeV

    SciTech Connect

    Roshchenko, V. A. Piksaikin, V. M. Korolev, G. G.; Egorov, A. S.

    2010-06-15

    The energy dependence of the relative abundances of delayed neutrons and the energy dependence of the half-lives of their precursors in the neutron-induced fission of {sup 232}Th nuclei in the energy range 3.2-17.9 MeV were measured for the first time. A systematics of the time features of delayed neutrons is developed. This systematics makes it possible to estimate the half-life of delayed-neutron precursors as a function of the nucleonic composition of fissile nuclei by using a single parameter set for all nuclides. The energy dependence of the partial cross sections for emissive fission in the reaction {sup 232}Th(n, f) was analyzed on the basis of data obtained for the relative abundances of delayed neutrons and the aforementioned half-lives and on the basis of the created systematics of the time features of delayed neutrons. It was shown experimentally for the first time that the decrease in the cross section after the reaction threshold in the fission of {sup 232}Th nuclei (it has a pronounced first-chance plateau) is not an exclusion among the already studied uranium, plutonium, and curium isotopes and complies with theoretical predictions obtained for the respective nuclei with allowance for shell, superfluid, and collective effects in the nuclear-level density and with allowance for preequilibrium neutron emission

  15. Statistical and evaporation models for the neutron emission energy spectrum in the center-of-mass system from fission fragments

    NASA Astrophysics Data System (ADS)

    Kawano, T.; Talou, P.; Stetcu, I.; Chadwick, M. B.

    2013-09-01

    The neutron emission energy spectra in the CMS (center-of-mass) frame from two compound nuclei produced by fission are studied. The neutron spectra calculated with the Hauser-Feshbach statistical model are compared with the evaporation theory, and the definition of the temperature is revisited. Using the Monte Carlo technique we average the CMS neutron spectra from many fission fragments to construct the representative CMS spectrum from both the light and heavy fragments. The CMS spectra for each fission fragment pair are also converted into the laboratory frame to calculate the total prompt fission neutron spectrum that can be observed experimentally. This is compared to measured laboratory data for thermal neutron induced fission on 235U. We show that the Hauser-Feshbach calculation gives a different spectrum shape than the Madland-Nix model calculation.

  16. LICORNE: A new and unique facility for producing intense, kinematically focused neutron beams at the IPN Orsay

    NASA Astrophysics Data System (ADS)

    Wilson, J. N.; Lebois, M.; Halipre, P.; Leniau, B.; Matea, I.; Verney, D.; Oberstedt, S.; Billnert, R.; Oberstedt, A.; Georgiev, G.; Ljungvall, J.

    2013-12-01

    LICORNE is a new neutron source recently installed at the tandem accelerator of the Institut de Physique Nucléaire d'Orsay, where a Li7-beam is used to bombard a hydrogen-containing target to produce an intense forward-directed neutron beam. The directionality of the beam, which is the unique characteristic of LICORNE, will permit the installation of γ-ray detectors dedicated to the investigation of fission fragment de-excitation which are unimpeded by neutrons from the source. A first experimental program will focus on the measurement of prompt γ-ray emission in the neutron-induced fission of fertile and fissile isotopes at incident neutron energies relevant for the core design of Generation-IV nuclear reactors. Other potential uses of the LICORNE facility for both fundamental and applied physics research are also presented.

  17. Simulation experiments for gamma-ray mapping of planetary surfaces: Scattering of high-energy neutrons

    NASA Technical Reports Server (NTRS)

    Brueckner, J.; Englert, P.; Reedy, R. C.; Waenke, H.

    1986-01-01

    The concentration and distribution of certain elements in surface layers of planetary objects specify constraints on models of their origin and evolution. This information can be obtained by means of remote sensing gamma-ray spectroscopy, as planned for a number of future space missions, i.e., Mars, Moon, asteroids, and comets. To investigate the gamma-rays made by interactions of neutrons with matter, thin targets of different composition were placed between a neutron-source and a high-resolution germanium spectrometer. Gamma-rays in the range of 0.1 to 8 MeV were accumulated. In one set of experiments a 14-MeV neutron generator using the T(d,n) reaction as neutron-source was placed in a small room. Scattering in surrounding walls produced a spectrum of neutron energies from 14 MeV down to thermal. This complex neutron-source induced mainly neutron-capture lines and only a few scattering lines. As a result of the set-up, there was a considerable background of discrete lines from surrounding materials. A similar situation exists under planetary exploration conditions: gamma-rays are induced in the planetary surface as well as in the spacecraft. To investigate the contribution of neutrons with higher energies, an experiment for the measurement of prompt gamma radiation was set up at the end of a beam-line of an isochronous cyclotron.

  18. Prompt Planetesimal Formation beyond the Snow Line

    NASA Astrophysics Data System (ADS)

    Armitage, Philip J.; Eisner, Josh A.; Simon, Jacob B.

    2016-09-01

    We develop a simple model to predict the radial distribution of planetesimal formation. The model is based on the observed growth of dust to millimeter-sized particles, which drift radially, pile-up, and form planetesimals where the stopping time and dust-to-gas ratio intersect the allowed region for streaming instability-induced gravitational collapse. Using an approximate analytic treatment, we first show that drifting particles define a track in metallicity–stopping time space whose only substantial dependence is on the disk’s angular momentum transport efficiency. Prompt planetesimal formation is feasible for high particle accretion rates (relative to the gas, {\\dot{M}}p/\\dot{M}≳ 3× {10}-2 for α ={10}-2), which could only be sustained for a limited period of time. If it is possible, it would lead to the deposition of a broad and massive belt of planetesimals with a sharp outer edge. Numerically including turbulent diffusion and vapor condensation processes, we find that a modest enhancement of solids near the snow line occurs for centimeter-sized particles, but that this is largely immaterial for planetesimal formation. We note that radial drift couples planetesimal formation across radii in the disk, and suggest that considerations of planetesimal formation favor a model in which the initial deposition of material for giant planet cores occurs well beyond the snow line.

  19. A delayed neutron technique for measuring induced fission rates in fresh and burnt LWR fuel

    NASA Astrophysics Data System (ADS)

    Jordan, K. A.; Perret, G.

    2011-04-01

    The LIFE@PROTEUS program at the Paul Scherrer Institut is being undertaken to characterize the interfaces between burnt and fresh fuel assemblies in modern LWRs. Techniques are being developed to measure fission rates in burnt fuel following re-irradiation in the zero-power PROTEUS research reactor. One such technique utilizes the measurement of delayed neutrons. To demonstrate the feasibility of the delayed neutron technique, fresh and burnt UO 2 fuel samples were irradiated in different positions in the PROTEUS reactor, and their neutron outputs were recorded shortly after irradiation. Fission rate ratios of the same sample irradiated in two different positions (inter-positional) and of two different samples irradiated in the same position (inter-sample) were derived from the measurements and compared with Monte Carlo predictions. Derivation of fission rate ratios from the delayed neutron measured signal requires correcting the signal for the delayed neutron source properties, the efficiency of the measurement setup, and the time dependency of the signal. In particular, delayed neutron source properties strongly depend on the fissile and fertile isotopes present in the irradiated sample and must be accounted for when deriving inter-sample fission rate ratios. Measured inter-positional fission rate ratios generally agree within 1σ uncertainty (on the order of 1.0%) with the calculation predictions. For a particular irradiation position, however, a bias of about 2% is observed and is currently under investigation. Calculated and measured inter-sample fission rate ratios have C/E values deviating from unity by less than 1% and within 2σ of the statistical uncertainties. Uncertainty arising from delayed neutron data is also assessed, and is found to give an additional 3% uncertainty factor. The measurement data indicate that uncertainty is overestimated.

  20. Prompt processes in heavy ion reactions

    SciTech Connect

    Blann, M.; Remington, B.A.

    1987-12-01

    We test a relaxation model based on two body nucleon-nucleon scattering processes to interpret phenomena observed in heavy ion reactions. We use the Boltzmann Master Equation to accomplish this. By assuming that the projectile nucleons partition the total excitation with equal a-priori probability of all configurations, we are able to reproduce several sets of neutron spectra from /sup 20/Ne and /sup 12/C induced reactions on /sup 165/Ho and from reactions of /sup 40/Ar or /sup 40/Ca. We point out ambiguities in deducing angle-integrated energy spectra from double differential spectra. With no additional free parameters, our model successfully reproduces a large body of high energy ..gamma..-ray spectra by assuming an incoherent n-p-bremsstrahlung mechanism. 45 refs., 13 figs.

  1. From radiation-induced chromosome damage to cell death: modelling basic mechanisms and applications to boron neutron capture therapy.

    PubMed

    Ballarini, F; Bortolussi, S; Clerici, A M; Ferrari, C; Protti, N; Altieri, S

    2011-02-01

    Cell death is a crucial endpoint in radiation-induced biological damage: on one side, cell death is a reference endpoint to characterise the action of radiation in biological targets; on the other side, any cancer therapy aims to kill tumour cells. Starting from Lea's target theory, many models have been proposed to interpret radiation-induced cell killing; after briefly discussing some of these models, in this paper, a mechanistic approach based on an experimentally observed link between chromosome aberrations and cell death was presented. More specifically, a model and a Monte Carlo code originally developed for chromosome aberrations were extended to simulate radiation-induced cell death applying an experimentally observed one-to-one relationship between the average number of 'lethal aberrations' (dicentrics, rings and deletions) per cell and -ln S, S being the fraction of surviving cells. Although such observation was related to X rays, in the present work, the approach was also applied to protons and alpha particles. A good agreement between simulation outcomes and literature data provided a model validation for different radiation types. The same approach was then successfully applied to simulate the survival of cells enriched with boron and irradiated with thermal neutrons at the Triga Mark II reactor in Pavia, to mimic a typical treatment for boron neutron capture therapy. PMID:21159746

  2. Neutron yields for reactions induced by 120 GeV protons on thick copper target

    SciTech Connect

    Kajimoto, Tsuyoshi; Sanami, Toshiya; Iwamoto, Yosuke; Shigyo, Nobuhiro; Hagiwara, Masayuki; Saitoh, Kiwamu; Nakashima, Hiroshi; Ishibashi, Kenji; Lee, Hee-Seock; Ramberg, Eric; Coleman, Richard; /Fermilab

    2011-02-01

    We developed an experimental method to measure neutron energy spectrum for 120-GeV protons on a thick copper target at Fermilab Test Beam Facility (FTBF). The spectrum in the energy range from 16 to 1600 MeV was obtained for 60-cm long copper target by time-of-flight technique with an NE213 scintillator and 5.5-m flight path. Energy spectra of neutrons generated from an interaction with beam and materials are important to design shielding structure of high energy accelerators. Until now, the energy spectra for the incident energy up to 3 GeV have been measured by several groups, Ishibashi et al., Amian et al., and Leray et al. In the energy region above 3 GeV, few experimental data are available because of small number of facilities for neutron experiment. On the other hand, concerning simulation codes, theoretical models for particle generation and transportation are switched from intermediate to high energy one around this energy. The spectra calculated by the codes have not been examined using experimental data. In shielding experiments using 120 GeV hadron beam, experimental data shows systematic differences from calculations. Hagiwara et al. have measured leakage neutron spectra behind iron and concrete shield from 120 GeV proton on target at anti-proton target station in Fermilab by using Bonner Spheres with unfolding technique. In CERN, Nakao et al reported experimental results of neutron spectra behind iron and concrete wall from 120 GeV/c proton and pion mixed beam on copper by using NE213 liquid scintillators with unfolding technique. Both of the results reported systematic discrepancies between experimental and calculation results. Therefore, experimental data are highly required to verify neutron production part of calculations. In this study, we developed an experimental method to measure neutron energy spectrum for 120 GeV proton on target. The neutron energy was determined using time-of-flight technique. We used the Fermilab Test Beam Facility (FTBF

  3. Protactinium neutron-induced fission up to 200 MeV

    NASA Astrophysics Data System (ADS)

    Maslov, V.

    2010-03-01

    The theoretical evaluation of 230-233Pa(n,F) cross sections is based on direct data, 230-234Pa fission probabilities and ratios of fission probabilities in first-chance and emissive fission domains, surrogate for neutroninduced fission. First chance fission cross sections trends of Pa are based on consistent description of 232Th(n,F), 232Th(n,2n) and 238U(n,F), 238U(n,xn) data, supported by the ratio surrogate data by Burke et al., 2006, for the 237U(n,F) reaction. Ratio surrogate data on fission probabilities of 232Th(6 Li,4 He)234Pa and 232 Th(6 Li,d)236U by Nayak et al., 2008, support the predicted 233Pa(n, F) cross section at En=11.5-16.5 MeV. The predicted trends of 230-232Pa(n, F) cross section up to En=20 MeV, are consistent with fissilities of Pa nuclides, extracted by 232Th(p,F) (Isaev et al., 2008) and 232Th(p,3n) (Morgenstern et al., 2008) data analysis. The excitation energy and nucleon composition dependence of the transition from asymmetric to symmetric scission for fission observables of Pa nuclei is defined by analysis of p-induced fission of 232Th at Ep=1-200 MeV. Predominantly symmetric fission in 232Th(p,F) at En( p)=200 MeV as revealed by experimental branching ratios (Dujvestijn et al., 1999) is reproduced. Steep transition from asymmetric to symmetric fission with increase of nucleon incident energy is due to fission of neutron-deficient Pa (A≤229) nuclei. A structure of the potential energy surface (a drop of f f symmetric and asymmetric fission barriers difierence (EfSYM - EfASYM) from ~3.5 MeV to ~1 MeV) of N-deficient Pa nuclides (A≤226) and available phase space at outer fission saddles, are shown to be responsible for the sharp increase with En( p) of the symmetric fission component contribution for 232Th(p,F) and 230-233 Pa(n, F) reactions. That is a strong evidence of emissive fission nature of moderately excited Pa nuclides, reliably quantified only up to En( p)~20(30) MeV. Predicted fission cross section of 232Pa(n,F) coincides

  4. Calculations of Neutron- and Proton-Induced Reactions up to 200 MeV for Target 238U

    SciTech Connect

    Yu Hongwei; Zhao Zhixiang; Cai Chonghai

    2005-05-24

    The calculations of neutron- and proton-induced reaction up to 200 MeV for target 238U are performed; the calculated results are generally in good agreement with experimental data, and the physics is rational. The theoretical framework consists of the spherical optical model, intranuclear cascade mechanism for nucleon emission based on empirical formula, preequilibrium emission theory based on exciton model, evaporation model, and Hauser-Feshbach statistical theory with a width fluctuation correction. The fission widths are calculated using the Bohr-Wheeler formula.

  5. A Monte Carlo simulation of the fission chambers neutron-induced pulse shape using the GARFIELD suite

    NASA Astrophysics Data System (ADS)

    Filliatre, P.; Jammes, C.; Geslot, B.; Veenhof, R.

    2012-06-01

    A computation route that simulates the neutron-induced charge spectrum and pulse shape of a fission chamber is presented. It is based on the GARFIELD suite, and makes use of the MAGBOLTZ and SRIM codes. It allows the simulation of the signal in the current and Campbelling modes. Computations made with several fission chambers exemplify the possibilities of the route. A good qualitative agreement is obtained when comparing the results with the scarce experimental data available to date. After a further experimental qualification, this route will improve the design of fission chambers by assessing its overall sensitivity.

  6. Measurement and analysis of radioactivity induced in steels and a vanadium alloy by 14-MeV neutrons

    NASA Astrophysics Data System (ADS)

    Richter, D.; Forrest, R. A.; Freiesleben, H.; Kovalchuk, Va. D.; Kovalchuk D, Vi.; Markovskij, D. V.; Seidel, K.; Tereshkin, V. I.; Unholzer, S.

    2000-12-01

    Samples of the structural material of the International Thermonuclear Experimental Reactor (SS316), of the low-activation steels MANET and F82H, and of the vanadium alloy V4Ti4Cr were irradiated with D-T fusion neutrons. The radioactivities induced were determined after irradiation several times during decay by γ-spectroscopy. The results were analysed with the European Activation System (EASY-97). In order to validate EASY-97, the total activities of the samples are compared, and ratios of calculated-to-experimental values for the individual activities are derived and discussed.

  7. T invariance and T-odd asymmetries for the cold-polarized-neutron-induced fission of nonoriented nuclei

    SciTech Connect

    Kadmensky, S. G.; Bunakov, V. E.; Titova, L. V.

    2014-12-15

    It is shown that the coefficients D{sup exp} for all T-odd asymmetries observed experimentally in the cross sections for the reactions of cold-polarized-neutron-induced fission of nonoriented target nuclei (which involves the emission of prescission and evaporated particles) comply in shape and scale with the coefficients D{sup theor} calculated for the analogous asymmetries on the basis of quantum-mechanical nuclear-fission theory for T-invariant Hamiltonians of fissile systems. It is also shown that the asymmetries in question arise upon taking into account the effect of (i) the interference between the fission amplitudes of s- and p-wave resonances of a polarized fissile compound nucleus formed in the aforementioned reactions; (ii) the collective rotation of the compound nucleus in question (this rotation entails a change in the angular distributions of fission fragments and third particles); and (iii) the wriggling vibrations of this compound nucleus in the vicinity of its scission point, which lead to the appearance of high aligned spins of fission fragments, with the result that the emission of neutrons and photons evaporated from these fragments becomes anisotropic. The possible contribution of T-noninvariant interactions to the formation of the T-odd asymmetries under analysis is estimated by using the results obtained in experimentally testing the detailed-balance principle, (P-A) theorem, and T invariance of cross sections for elastic proton-proton and proton-neutron scattering.

  8. Neutron-induced transmutation reactions in 237Np, 238Pu, and 239Pu at the massive natural uranium spallation target

    NASA Astrophysics Data System (ADS)

    Zavorka, L.; Adam, J.; Baldin, A. A.; Caloun, P.; Chilap, V. V.; Furman, W. I.; Kadykov, M. G.; Khushvaktov, J.; Pronskikh, V. S.; Solnyshkin, A. A.; Sotnikov, V.; Stegailov, V. I.; Suchopar, M.; Tsoupko-Sitnikov, V. M.; Tyutyunnikov, S. I.; Voronko, V.; Vrzalova, J.

    2015-04-01

    Transmutation reactions in the 237Np, 238Pu, and 239Pu samples were investigated in the neutron field generated inside a massive (m = 512 kg) natural uranium spallation target. The uranium target assembly QUINTA was irradiated with the deuteron beams of kinetic energy 2, 4, and 8 GeV provided by the Nuclotron accelerator at the Joint Institute for Nuclear Research (JINR) in Dubna. The neutron-induced transmutation of the actinide samples was measured off-line by implementing methods of gamma-ray spectrometry with HPGe detectors. Results of measurement are expressed in the form of both the individual reaction rates and average fission transmutation rates. For the purpose of validation of radiation transport programs, the experimental results were compared with simulations of neutron production and distribution performed by the MCNPX 2.7 and MARS15 codes employing the INCL4-ABLA physics models and LAQGSM event generator, respectively. In general, a good agreement between the experimental and calculated reaction rates was found in the whole interval of provided beam energies.

  9. Neutron scattering studies in the actinide region

    SciTech Connect

    Beghian, L.E.; Kegel, G.H.R.

    1991-08-01

    During the report period we have investigated the following areas: Neutron elastic and inelastic scattering measurements on {sup 14}N, {sup 181}Ta, {sup 232}Th, {sup 238}U and {sup 239}Pu; Prompt fission spectra for {sup 232}Th, {sup 235}U, {sup 238}U and {sup 239}Pu; Theoretical studies of neutron scattering; Neutron filters; New detector systems; and Upgrading of neutron target assembly, data acquisition system, and accelerator/beam-line apparatus.

  10. Monte Carlo simulation of moderator and reflector in coal analyzer based on a D-T neutron generator.

    PubMed

    Shan, Qing; Chu, Shengnan; Jia, Wenbao

    2015-11-01

    Coal is one of the most popular fuels in the world. The use of coal not only produces carbon dioxide, but also contributes to the environmental pollution by heavy metals. In prompt gamma-ray neutron activation analysis (PGNAA)-based coal analyzer, the characteristic gamma rays of C and O are mainly induced by fast neutrons, whereas thermal neutrons can be used to induce the characteristic gamma rays of H, Si, and heavy metals. Therefore, appropriate thermal and fast neutrons are beneficial in improving the measurement accuracy of heavy metals, and ensure that the measurement accuracy of main elements meets the requirements of the industry. Once the required yield of the deuterium-tritium (d-T) neutron generator is determined, appropriate thermal and fast neutrons can be obtained by optimizing the neutron source term. In this article, the Monte Carlo N-Particle (MCNP) Transport Code and Evaluated Nuclear Data File (ENDF) database are used to optimize the neutron source term in PGNAA-based coal analyzer, including the material and shape of the moderator and neutron reflector. The optimized targets include two points: (1) the ratio of the thermal to fast neutron is 1:1 and (2) the total neutron flux from the optimized neutron source in the sample increases at least 100% when compared with the initial one. The simulation results show that, the total neutron flux in the sample increases 102%, 102%, 85%, 72%, and 62% with Pb, Bi, Nb, W, and Be reflectors, respectively. Maximum optimization of the targets is achieved when the moderator is a 3-cm-thick lead layer coupled with a 3-cm-thick high-density polyethylene (HDPE) layer, and the neutron reflector is a 27-cm-thick hemispherical lead layer. PMID:26325583

  11. Investigation of the field-induced ferromagnetic phase transition in spin-polarized neutron matter: A lowest order constrained variational approach

    SciTech Connect

    Bordbar, G. H.; Rezaei, Z.; Montakhab, Afshin

    2011-04-15

    In this article, the lowest order constrained variational method is used to investigate the magnetic properties of spin-polarized neutron matter in the presence of strong magnetic field at zero temperature employing the AV{sub 18} potential. Our results indicate that a ferromagnetic phase transition is induced by a strong magnetic field with strength greater than 10{sup 18} G, leading to a partial spin polarization of the neutron matter. It is also shown that the equation of state of neutron matter in the presence of a magnetic field is stiffer than in the absence of a magnetic field.

  12. Tables of Neutron-Induced Fission Cross Section for Various Pu, U, and Th Isotopes, Deduced from Measured Fission Probabilites

    SciTech Connect

    Younes, W; Britt, H C

    2003-03-31

    Cross sections for neutron-induced fission of {sup 231,233}Th, {sup 234,235,236,237,239}U, and {sup 240,241,243}Pu are presented in tabular form for incident neutron energies of 0.1 {le} E{sub n}(MeV) {le} 2.5. The cross sections were obtained by converting measured fission probabilities from (t,pf) reactions on mass-A targets to (n,f) cross sections on mass-A + 1 neutron targets, by using modeling to compensate for the differences in the reaction mechanisms. Data from Britt et al. were used for the {sup 234}U(t,pf) reaction, from Cramer et al. for the {sup 230,232}Th(t,pf), {sup 236,238}U(t,pf), and {sup 240,242}Pu(t,pf) reactions, and from Britt et al. for the {sup 233,235}U(t,pf) and {sup 239}Pu(t,pf) reactions. The fission probabilities P{sub (t,pf)}(E{sub x}), measured as a function of excitation energy E{sub x} of the compound system formed by the (t,p) reaction, are listed in the tables with the corresponding deduced cross sections as a function of incident neutron energy E{sub n}, {sigma}{sub (n,f)}(E{sub n}). The excitation energy and incident neutron energy are related by E{sub x} = E{sub n} + B{sub n}, where B{sub n}, where B{sub n} is the neutron binding energy. Comparison with ENDF/B-VI evaluations of the well-measured {sup 234,235,236}U(n,f) and {sup 240,241}Pu(n,f) cross sections confirms the accuracy of the present results within a 10% standard deviation above E{sub n} = 1 MeV. Below E{sub n} = 1 MeV, localized deviations of at most {+-} 20% are observed.

  13. Observation of Gamma Irradiation-Induced Suppression of Reversed Annealing in Neutron Irradiated MCZ Si Detectors

    SciTech Connect

    Li, Z.; Gul, R.; Harkonen, J.; Kierstead, J.; Metcalfe, J.; Seidel, S.

    2009-02-06

    For the development of radiation-hard Si detectors for the SiD BeamCal program for the future ILC (International Linear Collider), n-type MCZ Si detectors have been irradiated first by fast neutrons to flueneces of 1.5 x 1014 and 3 x 1014 neq/cm2, and then by gamma up to 500 Mrad. The motivation of this mixed radiation project is to develop a Si detector that can utilize the gamma/electron radiation that exists in the ICL radiation environment, which also includes neutrons. By using the positive space charge (SC) created by gamma radiation in MCZ Si detectors, one can cancel the negative space charge created by neutrons, thus reducing the overall/net space charge density and therefore the full depletion voltage of the detector.

  14. Modeling of neutron induced backgrounds in x-ray framing cameras.

    PubMed

    Hagmann, C; Izumi, N; Bell, P; Bradley, D; Conder, A; Eckart, M; Khater, H; Koch, J; Moody, J; Stone, G

    2010-10-01

    Fast neutrons from inertial confinement fusion implosions pose a severe background to conventional multichannel plate (MCP)-based x-ray framing cameras for deuterium-tritium yields >10(13). Nuclear reactions of neutrons in photosensitive elements (charge coupled device or film) cause some of the image noise. In addition, inelastic neutron collisions in the detector and nearby components create a large gamma pulse. The background from the resulting secondary charged particles is twofold: (1) production of light through the Cherenkov effect in optical components and by excitation of the MCP phosphor and (2) direct excitation of the photosensitive elements. We give theoretical estimates of the various contributions to the overall noise and present mitigation strategies for operating in high yield environments. PMID:21034042

  15. Measurements of Neutron Induced Cross Sections at the Oak Ridge Electron Linear Accelerator

    SciTech Connect

    Guber, K.H.; Harvey, J.A.; Hill, N.W.; Koehler, P.E.; Leal, L.C.; Sayer, R.O.; Spencer, R.R.

    1999-09-20

    We have used the Oak Ridge Electron Linear Accelerator (ORELA) to measure neutron total and the fission cross sections of 233U in the energy range from 0.36 eV to ~700 keV. We report average fission and total cross sections. Also, we measured the neutron total cross sections of 27Al and Natural chlorine as well as the capture cross section of Al over an energy range from 100 eV up to about 400 keV.

  16. Radiation cataractogenesis induced by neutron or gamma irradiation in the rat lens is reduced by vitamin E

    SciTech Connect

    Ross, W.M.; Creighton, M.O.; Trevithick, J.R. )

    1990-09-01

    Although cataract of the eye lens is a known late effect of ionizing radiation exposure, most of the experimental work to date has concentrated on single, acute high doses or multiple, fractionated, chronic exposures. Many papers have dealt with biochemical alterations in metabolism and cellular components, with microscopic and electron microscopic lesions to the epithelial and cortical layers, and with clinical cataract formation. However, the minimum cataractogenic dose for rats has for many years been considered to be about 2 Gy for a single, acute dose of low LET radiation. Our purpose in designing this pilot study was three fold: firstly, to determine whether any physical damage could be detected after low, acute exposure to neutron radiation (10 and 100 cGy); secondly, to compare the relative effectiveness of fast (14 MeV) neutrons with gamma-rays; and thirdly, to investigate the possibility that vitamin E could protect the lenses from radiation damage. The results revealed that morphological damage was already discernible within minutes after exposure to neutrons or gamma-rays, that it became greater after 24 hours, that neutrons were more damaging than gamma-rays, and that vitamin E could effectively reduce the cataractogenic damage induced by ionizing radiation. Control, non-irradiated lenses with or without vitamin E, either in vivo or in vitro, showed no damage. Also, it appeared that in vitro irradiation was more damaging to lenses than in vivo irradiation, so this culture technique may prove to be a sensitive tool for assessing early damage caused by ionizing radiation.

  17. Measurement of neutron energy spectra and neutron dose rates from 7Li(p,n)7Be reaction induced on thin LiF target

    NASA Astrophysics Data System (ADS)

    Atanackovic, Jovica; Matysiak, Witold; Dubeau, Jacques; Witharana, Sampath; Waker, Anthony

    2015-02-01

    The measurements of neutron energy spectra and neutron dose rates were performed using the KN Van de Graaff accelerator, located at the McMaster University Accelerator Laboratory (MAL). Protons were accelerated on the thin lithium fluoride (LiF) target and produced mono-energetic neutrons which were measured using three different spectrometers: Bonner Sphere Spectrometer (BSS), Nested Neutron Spectrometer (NNS), and Rotational Proton Recoil Spectrometer (ROSPEC). The purpose of this work is (1) measurement and quantification of low energy accelerator neutron fields in terms of neutron fluence and dose, (2) comparison of results obtained by three different instruments, (3) comparison of measurements with Monte Carlo simulations based on theoretical neutron yields from 7Li(p,n)7Be nuclear reaction, and (4) comparison of results obtained using different neutron spectral unfolding methods. The nominal thickness of the LiF target used in the experiment was 50 μg /cm2, which corresponds to the linear thickness of 0.19 μm and results in approximately 6 keV energy loss for the proton energies used in the experiment (2.2, 2.3, 2.4 and 2.5 MeV). For each of the proton energies, neutron fluence per incident proton charge was measured and several dosimetric quantities of interest in radiation protection were derived. In addition, theoretical neutron yield calculations together with the results of Monte Carlo (MCNP) modeling of the neutron spectra are reported. Consistent neutron fluence spectra were obtained with three detectors and good agreement was observed between theoretically calculated and measured neutron fluences and derived dosimetric quantities for investigated proton energies at 2.3, 2.4 and 2.5 MeV. In the case of 2.2 MeV, some plausibly explainable discrepancies were observed.

  18. 10 CFR 15.61 - Prompt referral.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... shall promptly refer debts that are subject to aggressive collection activity (as described in subpart B..., consistent with the NRC's aggressive collection activity and well within the one year of the NRC's...

  19. 45 CFR 1701.5 - Prompt response.

    Code of Federal Regulations, 2013 CFR

    2013-10-01

    ... INFORMATION SCIENCE DISCLOSURE OF INFORMATION § 1701.5 Prompt response. (a) Within ten days (excluding... ten-day period, or the last extension thereof, the requester may deem his request denied, and...

  20. 45 CFR 1701.5 - Prompt response.

    Code of Federal Regulations, 2012 CFR

    2012-10-01

    ... INFORMATION SCIENCE DISCLOSURE OF INFORMATION § 1701.5 Prompt response. (a) Within ten days (excluding... ten-day period, or the last extension thereof, the requester may deem his request denied, and...