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Sample records for nonlinear wave-packet interferometry

  1. Nonlinear wave packet interferometry and molecular state reconstruction

    NASA Astrophysics Data System (ADS)

    Humble, Travis Selby

    Nonlinear wave packet interferometry (WPI) uses two phase-locked pulse-pairs to excite a molecular electronic population and measures those contributions arising from a one-pulse nuclear wave packet overlapping with a three-pulse nuclear wave packet. The interferogram quantifies the wave-packet interference at the probability-amplitude level and, with knowledge of the three-pulse (reference) wave packets, enables reconstruction of the one-pulse (target) wave packet. In one-color nonlinear WPI, both pulse-pairs resonate with the same electronic transition and the interferogram measures a sum of wave-packet overlaps. Experimental conditions often minimize mixing of these overlaps and hence permit molecular state reconstruction, as demonstrated by numerical calculations for model harmonic and photodissociative systems. Yet, a one-color reconstruction technique requires information about the Hamiltonian under which the target and reference states propagate. The latter knowledge obviates the practical need for experimental state determination, since computational methods are then a viable, alternative solution. Two-color nonlinear WPI, in which the pulse-pairs drive different electronic transitions, circumvents the need for information about the target-state Hamiltonian by using an auxiliary electronic level for preparing the reference states. Furthermore, in a two-color experiment, the interferogram measures a single wave-packet overlap, definitely identifying the information necessary for molecular state reconstruction. These features suggest two-color nonlinear WPI could serve as a diagnostic tool for identifying optically-controlled, yet unknown, molecular dynamics. Simulations for model systems and the lithium dimer demonstrate that target states can be reconstructed in the presence of signal noise, thermal mixtures, and rovibrational coupling and in the absence of information about the target-state Hamiltonian. In the presence of electronic-energy transfer, the

  2. Molecular wave packet interferometry and quantum entanglement

    NASA Astrophysics Data System (ADS)

    Martínez-Galicia, Ricardo; Romero-Rochín, Víctor

    2005-03-01

    We study wave packet interferometry (WPI) considering the laser pulse fields both classical and quantum mechanically. WPI occurs in a molecule after subjecting it to the interaction with a sequence of phase-locked ultrashort laser pulses. Typically, the measured quantity is the fluorescence of the molecule from an excited electronic state. This signal has imprinted the interference of the vibrational wave packets prepared by the different laser pulses of the sequence. The consideration of the pulses as quantum entities in the analysis allows us to study the entanglement of the laser pulse states with the molecular states. With a simple model for the molecular system, plus several justified approximations, we solve for the fully quantum mechanical molecule-electromagnetic field state. We then study the reduced density matrices of the molecule and the laser pulses separately. We calculate measurable corrections to the case where the fields are treated classically.

  3. Calculations of nonlinear wave-packet interferometry signals in the pump-probe limit as tests for vibrational control over electronic excitation transfer

    NASA Astrophysics Data System (ADS)

    Biggs, Jason D.; Cina, Jeffrey A.

    2009-12-01

    The preceding paper [J. D. Biggs and J. A. Cina, J. Chem. Phys. 131, 224101 (2009)] (referred to here as Paper 1), describes a strategy for externally influencing the course of short-time electronic excitation transfer (EET) in molecular dimers and observing the process by nonlinear wave-packet interferometry (nl-WPI). External influence can, for example, be exerted by inducing coherent intramolecular vibration in one of the chromophores prior to short-pulse electronic excitation of the other. Within a sample of isotropically oriented dimers having a specified internal geometry, a vibrational mode internal to the acceptor chromophore can be preferentially driven by electronically nonresonant impulsive stimulated Raman (or resonant infrared) excitation with a short polarized "control" pulse. A subsequent electronically resonant polarized pump then preferentially excites the donor, and EET ensues. Paper 1 investigates control-pulse-influenced nl-WPI as a tool for the spectroscopic evaluation of the effect of coherent molecular vibration on excitation transfer, presenting general expressions for the nl-WPI difference signal from a dimer following the action of a control pulse of arbitrary polarization and shape. Electronic excitation is to be effected and its interchromophore transfer monitored by resonant pump and probe "pulses," respectively, each consisting of an optical-phase-controlled ultrashort pulse-pair having arbitrary polarization, duration, center frequency, and other characteristics. Here we test both the control strategy and its spectroscopic investigation—with some sacrifice of amplitude-level detail—by calculating the pump-probe difference signal. That signal is the limiting case of the control-influenced nl-WPI signal in which the two pulses in the pump pulse-pair coincide, as do the two pulses in the probe pulse-pair. We present calculated pump-probe difference signals for (1) a model excitation-transfer complex in which two equal-energy monomers

  4. Behavior of a Moist Kelvin Wave Packet with Nonlinear Heating.

    NASA Astrophysics Data System (ADS)

    Wang, Bin; Xue, Yan

    1992-04-01

    The effects of nonlinear (positive only or conditional) heating on moist Kelvin waves are examined with a simple equatorial zonal-plane model describing the gravest baroclinic mode.The unstable perturbation subject to nonlinear beating emerges as a wave packet. A typical amplifying, eastward-moving wave packet is characterized by an asymmetric structure: 1) the ascending branch (wet region) is much narrower than the two descending ones (dry regions); and 2) the circulation cell to the east of the wet region center is smaller and stronger than its counterpart to the west of the center. The wet-dry asymmetry is primarily caused by the nonlinear beating effect, while the east-west asymmetry is a result of the movement of the wave packet relative to mean flow. The existence of Newtonian cooling and Rayleigh friction enhances the structural asymmetries.The unstable wave packet is characterized by two zonal length scales: the ascending branch length (ABL) and total circulation extent (TCE). For a given basic state, the growth rate of a wave packet increases with decreasing ABL or TCE. However, up to a moderate growth rate (order of day1) the energy spectra of all wave packets are dominated by zonal wavenumber one regardless of ABL size. In particular, the slowly growing (low frequency) wave packets normally exhibit TCEs of planetary scale and ABLs of synoptic scale.Observed equatorial intraseasonal disturbances often display a narrow convection region in between two much broader dry regions and a total circulation of planetary scale. These structure and scale characteristics are caused by the effects of nonlinear heating and the cyclic geometry of the equator. It is argued that the unstable disturbance found in numerical experiments (e.g., Lau and Peng; Hayashi and Sumi) is a manifestation of the nonlinear wave packet.

  5. Atom interferometry using wave packets with constant spatial displacements

    SciTech Connect

    Su, Edward J.; Prentiss, Mara G.; Wu Saijun

    2010-04-15

    A standing-wave light-pulse sequence is demonstrated that places atoms into a superposition of wave packets with precisely controlled displacements that remain constant for times as long as 1 s. The separated wave packets are subsequently recombined, resulting in atom interference patterns that probe energy differences of {approx_equal}10{sup -34} J and can provide acceleration measurements that are insensitive to platform vibrations.

  6. Nonlinear Evolution of Alfvenic Wave Packets

    NASA Technical Reports Server (NTRS)

    Buti, B.; Jayanti, V.; Vinas, A. F.; Ghosh, S.; Goldstein, M. L.; Roberts, D. A.; Lakhina, G. S.; Tsurutani, B. T.

    1998-01-01

    Alfven waves are a ubiquitous feature of the solar wind. One approach to studying the evolution of such waves has been to study exact solutions to approximate evolution equations. Here we compare soliton solutions of the Derivative Nonlinear Schrodinger evolution equation (DNLS) to solutions of the compressible MHD equations.

  7. Using wave-packet interferometry to monitor the external vibrational control of electronic excitation transfer

    NASA Astrophysics Data System (ADS)

    Biggs, Jason D.; Cina, Jeffrey A.

    2009-12-01

    We investigate the control of electronic energy transfer in molecular dimers through the preparation of specific vibrational coherences prior to electronic excitation, and its observation by nonlinear wave-packet interferometry (nl-WPI). Laser-driven coherent nuclear motion can affect the instantaneous resonance between site-excited electronic states and thereby influence short-time electronic excitation transfer (EET). We first illustrate this control mechanism with calculations on a dimer whose constituent monomers undergo harmonic vibrations. We then consider the use of nl-WPI experiments to monitor the nuclear dynamics accompanying EET in general dimer complexes following impulsive vibrational excitation by a subresonant control pulse (or control pulse sequence). In measurements of this kind, two pairs of polarized phase-related femtosecond pulses following the control pulse generate superpositions of coherent nuclear wave packets in optically accessible electronic states. Interference contributions to the time- and frequency-integrated fluorescence signals due to overlaps among the superposed wave packets provide amplitude-level information on the nuclear and electronic dynamics. We derive the basic expression for a control-pulse-dependent nl-WPI signal. The electronic transition moments of the constituent monomers are assumed to have a fixed relative orientation, while the overall orientation of the complex is distributed isotropically. We include the limiting case of coincident arrival by pulses within each phase-related pair in which control-influenced nl-WPI reduces to a fluorescence-detected pump-probe difference experiment. Numerical calculations of pump-probe signals based on these theoretical expressions are presented in the following paper [J. D. Biggs and J. A. Cina, J. Chem. Phys. 131, 224302 (2009)].

  8. Nonlinear single Compton scattering of an electron wave packet

    NASA Astrophysics Data System (ADS)

    Angioi, A.; Mackenroth, F.; Di Piazza, A.

    2016-05-01

    Nonlinear single Compton scattering has been thoroughly investigated in the literature under the assumption that the electron initially has a definite momentum. Here, we study a more general initial state and consider the electron as a wave packet. In particular, we investigate the energy spectrum of the emitted radiation and show that, in typical experimental situations, some features of the spectra shown in previous works are almost completely washed out. Moreover, we show that, at comparable relative uncertainties, the one in the momentum of the incoming electron has a larger impact on the photon spectra at a fixed observation direction than the one on the laser frequency.

  9. Phase shifts and wave-packet displacements in neutron interferometry and a nondispersive, nondefocusing phase shifter

    SciTech Connect

    Lemmel, Hartmut; Wagh, Apoorva G.

    2010-09-15

    A phase shifter in neutron interferometry creates not only a phase shift but also a spatial displacement of the neutron wave packet, leading to a reduced interference contrast. This wave-packet displacement constitutes a major hindrance in measuring large phase shifts. Here we present a nondispersive configuration with two identical phase shifters placed on one path in successive gaps of a symmetric triple Laue (LLL) interferometer. As compared to a single phase shifter, the dual phase shifter generates double the phase shift, yet a net null displacement of the wave packet. The interferometer thus remains fully focused however large the phase shift or the incident wavelength spread, permitting a white incident neutron beam as in the case of a purely topological phase measurement. Misalignment angles of a monolithic nondispersive dual phase shifter are equal and opposite in the two gaps. Its phase therefore remains nondispersive over a much wider angular range and attains a minimum magnitude at the correct orientation, obviating the need to alternate the phase shifter between the two interferometer paths during its alignment. The setup is hence ideally suited for measuring neutron coherent scattering lengths to ultrahigh precision.

  10. Nonlinear dynamics of Airy-vortex 3D wave packets: emission of vortex light waves.

    PubMed

    Driben, Rodislav; Meier, Torsten

    2014-10-01

    The dynamics of 3D Airy-vortex wave packets is studied under the action of strong self-focusing Kerr nonlinearity. Emissions of nonlinear 3D waves out of the main wave packets with the topological charges were demonstrated. Because of the conservation of the total angular momentum, charges of the emitted waves are equal to those carried by the parental light structure. The rapid collapse imposes a severe limitation on the propagation of multidimensional waves in Kerr media. However, the structure of the Airy beam carrier allows the coupling of light from the leading, most intense peak into neighboring peaks and consequently strongly postpones the collapse. The dependence of the critical input amplitude for the appearance of a fast collapse on the beam width is studied for wave packets with zero and nonzero topological charges. Wave packets carrying angular momentum are found to be much more resistant to the rapid collapse. PMID:25360922

  11. Wave packet interferometry and quantum state reconstruction by acousto-optic phase modulation

    NASA Astrophysics Data System (ADS)

    Tekavec, Patrick F.; Dyke, Thomas R.; Marcus, Andrew H.

    2006-11-01

    Studies of wave packet dynamics often involve phase-selective measurements of coherent optical signals generated from sequences of ultrashort laser pulses. In wave packet interferometry (WPI), the separation between the temporal envelopes of the pulses must be precisely monitored or maintained. Here we introduce a new (and easy to implement) experimental scheme for phase-selective measurements that combines acousto-optic phase modulation with ultrashort laser excitation to produce an intensity-modulated fluorescence signal. Synchronous detection, with respect to an appropriately constructed reference, allows the signal to be simultaneously measured at two phases differing by 90°. Our method effectively decouples the relative temporal phase from the pulse envelopes of a collinear train of optical pulse pairs. We thus achieve a robust and high signal-to-noise scheme for WPI applications, such as quantum state reconstruction and electronic spectroscopy. The validity of the method is demonstrated, and state reconstruction is performed, on a model quantum system—atomic Rb vapor. Moreover, we show that our measurements recover the correct separation between the absorptive and dispersive contributions to the system susceptibility.

  12. Wave packet interferometry and quantum state reconstruction by acousto-optic phase modulation

    SciTech Connect

    Tekavec, Patrick F.; Dyke, Thomas R.; Marcus, Andrew H.

    2006-11-21

    Studies of wave packet dynamics often involve phase-selective measurements of coherent optical signals generated from sequences of ultrashort laser pulses. In wave packet interferometry (WPI), the separation between the temporal envelopes of the pulses must be precisely monitored or maintained. Here we introduce a new (and easy to implement) experimental scheme for phase-selective measurements that combines acousto-optic phase modulation with ultrashort laser excitation to produce an intensity-modulated fluorescence signal. Synchronous detection, with respect to an appropriately constructed reference, allows the signal to be simultaneously measured at two phases differing by 90 deg. Our method effectively decouples the relative temporal phase from the pulse envelopes of a collinear train of optical pulse pairs. We thus achieve a robust and high signal-to-noise scheme for WPI applications, such as quantum state reconstruction and electronic spectroscopy. The validity of the method is demonstrated, and state reconstruction is performed, on a model quantum system - atomic Rb vapor. Moreover, we show that our measurements recover the correct separation between the absorptive and dispersive contributions to the system susceptibility.

  13. Wave-Packet Interferometry and Molecular State Reconstruction: Spectroscopic Adventures on the Left-Hand Side of the Schrödinger Equation

    NASA Astrophysics Data System (ADS)

    Cina, Jeffrey A.

    2008-05-01

    This article summarizes theoretical studies of molecular state determination by wave-packet interferometry (WPI) and recounts some recent experimental applications of molecular WPI. Calculations predict that two-color nonlinear WPI data can be used to reconstruct a rovibronic target wave packet evolving under an incompletely characterized nuclear Hamiltonian. This can be accomplished by the isolation via phase cycling or wave-vector matching of an exhaustive collection of overlaps between the unknown target and the members of a family of reference wave packets whose form is known by construction. This review highlights recent experiments employing WPI to gain amplitude-level information about the photoexcited-state dynamics of small molecules in the gas phase and in rare-gas crystals. I briefly describe a new semiclassical theory for condensed-phase WPI and other coherence-spectroscopy measurements, such as time-resolved coherent anti-Stokes Raman scattering, and mention our initial studies of nonlinear WPI from electronic energy-transfer complexes.

  14. Phase-modulated electronic wave packet interferometry reveals high resolution spectra of free Rb atoms and Rb*He molecules.

    PubMed

    Bruder, Lukas; Mudrich, Marcel; Stienkemeier, Frank

    2015-10-01

    Phase-modulated wave packet interferometry is combined with mass-resolved photoion detection to investigate rubidium atoms attached to helium nanodroplets in a molecular beam experiment. The spectra of atomic Rb electronic states show a vastly enhanced sensitivity and spectral resolution when compared to conventional pump-probe wave packet interferometry. Furthermore, the formation of Rb*He exciplex molecules is probed and for the first time a fully resolved vibrational spectrum for transitions between the lowest excited 5Π3/2 and the high-lying electronic states 2(2)Π, 4(2)Δ, 6(2)Σ is obtained and compared to theory. The feasibility of applying coherent multidimensional spectroscopy to dilute cold gas phase samples is demonstrated in these experiments. PMID:26309123

  15. Wave-packet rectification in nonlinear electronic systems: A tunable Aharonov-Bohm diode

    PubMed Central

    Li, Yunyun; Zhou, Jun; Marchesoni, Fabio; Li, Baowen

    2014-01-01

    Rectification of electron wave-packets propagating along a quasi-one dimensional chain is commonly achieved via the simultaneous action of nonlinearity and longitudinal asymmetry, both confined to a limited portion of the chain termed wave diode. However, it is conceivable that, in the presence of an external magnetic field, spatial asymmetry perpendicular to the direction of propagation suffices to ensure rectification. This is the case of a nonlinear ring-shaped lattice with different upper and lower halves (diode), which is attached to two elastic chains (leads). The resulting device is mirror symmetric with respect to the ring vertical axis, but mirror asymmetric with respect to the chain direction. Wave propagation along the two diode paths can be modeled for simplicity by a discrete Schrödinger equation with cubic nonlinearities. Numerical simulations demonstrate that, thanks to the Aharonov-Bohm effect, such a diode can be operated by tuning the magnetic flux across the ring. PMID:24691462

  16. Wave-packet rectification in nonlinear electronic systems: a tunable Aharonov-Bohm diode.

    PubMed

    Li, Yunyun; Zhou, Jun; Marchesoni, Fabio; Li, Baowen

    2014-01-01

    Rectification of electron wave-packets propagating along a quasi-one dimensional chain is commonly achieved via the simultaneous action of nonlinearity and longitudinal asymmetry, both confined to a limited portion of the chain termed wave diode. However, it is conceivable that, in the presence of an external magnetic field, spatial asymmetry perpendicular to the direction of propagation suffices to ensure rectification. This is the case of a nonlinear ring-shaped lattice with different upper and lower halves (diode), which is attached to two elastic chains (leads). The resulting device is mirror symmetric with respect to the ring vertical axis, but mirror asymmetric with respect to the chain direction. Wave propagation along the two diode paths can be modeled for simplicity by a discrete Schrödinger equation with cubic nonlinearities. Numerical simulations demonstrate that, thanks to the Aharonov-Bohm effect, such a diode can be operated by tuning the magnetic flux across the ring. PMID:24691462

  17. Mesoscopic transport and interferometry with wave packets of ultracold atoms: Effects of quantum coherence and interactions

    SciTech Connect

    Das, Kunal K.

    2011-09-15

    We propose a way to simulate mesoscopic transport processes with counterpropagating wave packets of ultracold atoms in quasi-one-dimensional (1D) waveguides and show quantitative agreement with analytical results. The method allows the study of a broad range of transport processes at the level of individual modes, not possible in electronic systems. Typically suppressed effects of quantum coherence become manifest, along with the effects of tunable interactions, which can be used to develop a simpler type of sensitive atom interferometer.

  18. Wave packet dynamics for a non-linear Schrödinger equation describing continuous position measurements

    NASA Astrophysics Data System (ADS)

    Zander, C.; Plastino, A. R.; Díaz-Alonso, J.

    2015-11-01

    We investigate time-dependent solutions for a non-linear Schrödinger equation recently proposed by Nassar and Miret-Artés (NM) to describe the continuous measurement of the position of a quantum particle (Nassar, 2013; Nassar and Miret-Artés, 2013). Here we extend these previous studies in two different directions. On the one hand, we incorporate a potential energy term in the NM equation and explore the corresponding wave packet dynamics, while in the previous works the analysis was restricted to the free-particle case. On the other hand, we investigate time-dependent solutions while previous studies focused on a stationary one. We obtain exact wave packet solutions for linear and quadratic potentials, and approximate solutions for the Morse potential. The free-particle case is also revisited from a time-dependent point of view. Our analysis of time-dependent solutions allows us to determine the stability properties of the stationary solution considered in Nassar (2013), Nassar and Miret-Artés (2013). On the basis of these results we reconsider the Bohmian approach to the NM equation, taking into account the fact that the evolution equation for the probability density ρ =| ψ | 2 is not a continuity equation. We show that the effect of the source term appearing in the evolution equation for ρ has to be explicitly taken into account when interpreting the NM equation from a Bohmian point of view.

  19. Sorting photon wave packets using temporal-mode interferometry based on multiple-stage quantum frequency conversion

    NASA Astrophysics Data System (ADS)

    Reddy, D. V.; Raymer, M. G.; McKinstrie, C. J.

    2015-01-01

    All classical and quantum technologies that encode in and retrieve information from optical fields rely on the ability to selectively manipulate orthogonal field modes of light. Such manipulation can be achieved with high selectivity for polarization modes and transverse-spatial modes. For the time-frequency degree of freedom, this could efficiently be achieved for a limited choice of approximately orthogonal modes, i.e., nonoverlapping bins in time or frequency. We recently proposed a method that surmounts the selectivity barrier for sorting arbitrary orthogonal temporal modes [Opt. Lett. 39, 2924 (2014)., 10.1364/OL.39.002924] using cascaded interferometric quantum frequency conversion in nonlinear optical media. We call this method temporal-mode interferometry, as it has a close resemblance to the well-known separated-fields atomic interferometry method introduced by Ramsey. The method has important implications for quantum memories, quantum dense coding, quantum teleportation, and quantum key distribution. Here we explore the inner workings of the method in detail, and extend it to multiple stages with a concurrent asymptotic convergence of temporal-mode selectivity to unity. We also complete our analysis of pump-chirp compensation to counter pump-induced nonlinear phase modulation in four-wave mixing implementations.

  20. Exploring Divisibility and Summability of 'Photon' Wave Packets in Nonlinear Optical Phenomena

    NASA Technical Reports Server (NTRS)

    Prasad, Narasimha; Roychoudhuri, Chandrasekhar

    2009-01-01

    Formulations for second and higher harmonic frequency up and down conversions, as well as multi photon processes directly assume summability and divisibility of photons. Quantum mechanical (QM) interpretations are completely congruent with these assumptions. However, for linear optical phenomena (interference, diffraction, refraction, material dispersion, spectral dispersion, etc.), we have a profound dichotomy. Most optical engineers innovate and analyze all optical instruments by propagating pure classical electromagnetic (EM) fields using Maxwell s equations and gives only lip-service to the concept "indivisible light quanta". Further, irrespective of linearity or nonlinearity of the phenomena, the final results are always registered through some photo-electric or photo-chemical effects. This is mathematically well modeled by a quadratic action (energy absorption) relation. Since QM does not preclude divisibility or summability of photons in nonlinear & multi-photon effects, it cannot have any foundational reason against these same possibilities in linear optical phenomena. It implies that we must carefully revisit the fundamental roots behind all light-matter interaction processes and understand the common origin of "graininess" and "discreteness" of light energy.

  1. Controlled Splitting of an Atomic Wave Packet

    SciTech Connect

    Zhang, M.; Zhang, P.; Chapman, M. S.; You, L.

    2006-08-18

    We propose a simple scheme capable of adiabatically splitting an atomic wave packet using two independent translating traps. Implemented with optical dipole traps, our scheme allows a high degree of flexibility for atom interferometry arrangements and highlights its potential as an efficient and high fidelity atom optical beam splitter.

  2. Wave-Packet and Coherent Control Dynamics

    NASA Astrophysics Data System (ADS)

    Ohmori, Kenji

    2009-05-01

    This review summarizes progress in coherent control as well as relevant recent achievements, highlighting, among several different schemes of coherent control, wave-packet interferometry (WPI). WPI is a fundamental and versatile scenario used to control a variety of quantum systems with a sequence of short laser pulses whose relative phase is finely adjusted to control the interference of electronic or nuclear wave packets (WPs). It is also useful in retrieving quantum information such as the amplitudes and phases of eigenfunctions superposed to generate a WP. Experimental and theoretical efforts to retrieve both the amplitude and phase information are recounted. This review also discusses information processing based on the eigenfunctions of atoms and molecules as one of the modern and future applications of coherent control. The ultrafast coherent control of ultracold atoms and molecules and the coherent control of complex systems are briefly discussed as future perspectives.

  3. Particlelike wave packets in complex scattering systems

    NASA Astrophysics Data System (ADS)

    Gérardin, Benoît; Laurent, Jérôme; Ambichl, Philipp; Prada, Claire; Rotter, Stefan; Aubry, Alexandre

    2016-07-01

    A wave packet undergoes a strong spatial and temporal dispersion while propagating through a complex medium. This wave scattering is often seen as a nightmare in wave physics whether it be for focusing, imaging, or communication purposes. Controlling wave propagation through complex systems is thus of fundamental interest in many areas, ranging from optics or acoustics to medical imaging or telecommunications. Here, we study the propagation of elastic waves in a cavity and a disordered waveguide by means of laser interferometry. From the direct experimental access to the time-delay matrix of these systems, we demonstrate the existence of particlelike wave packets that remain focused in time and space throughout their complex trajectory. Due to their limited dispersion, their selective excitation will be crucially relevant for all applications involving selective wave focusing and efficient information transfer through complex media.

  4. Self-Interfering Wave Packets.

    PubMed

    Colas, David; Laussy, Fabrice P

    2016-01-15

    We study the propagation of noninteracting polariton wave packets. We show how two qualitatively different concepts of mass that arise from the peculiar polariton dispersion lead to a new type of particlelike object from noninteracting fields-much like self-accelerating beams-shaped by the Rabi coupling out of Gaussian initial states. A divergence and change of sign of the diffusive mass results in a "mass wall" on which polariton wave packets bounce back. Together with the Rabi dynamics, this yields propagation of ultrafast subpackets and ordering of a spacetime crystal. PMID:26824554

  5. Self-Interfering Wave Packets

    NASA Astrophysics Data System (ADS)

    Colas, David; Laussy, Fabrice P.

    2016-01-01

    We study the propagation of noninteracting polariton wave packets. We show how two qualitatively different concepts of mass that arise from the peculiar polariton dispersion lead to a new type of particlelike object from noninteracting fields—much like self-accelerating beams—shaped by the Rabi coupling out of Gaussian initial states. A divergence and change of sign of the diffusive mass results in a "mass wall" on which polariton wave packets bounce back. Together with the Rabi dynamics, this yields propagation of ultrafast subpackets and ordering of a spacetime crystal.

  6. Controlling plasmonic wave packets in silver nanowires.

    SciTech Connect

    Cao, L.; Nome, R.; Montgomery, J. M.; Gray, S. K.; Scherer, N. F.

    2010-09-01

    Three-dimensional finite-difference time-domain simulations were performed to explore the excitation of surface plasmon resonances in long silver (Ag) nanowires. In particular, we show that it is possible to generate plasmonic wave packets that can propagate along the nanowire by exciting superpositions of surface plasmon resonances. By using an appropriately chirped pulse, it is possible to transiently achieve localization of the excitation at the distal end of the nanowire. Such designed coherent superpositions will allow realizing spatiotemporal control of plasmonic excitations for enhancing nonlinear responses in plasmonic 'circuits'.

  7. Repulsive gravitational effect of a quantum wave packet and experimental scheme with superfluid helium

    NASA Astrophysics Data System (ADS)

    Xiong, Hongwei

    2015-08-01

    We consider the gravitational effect of quantum wave packets when quantum mechanics, gravity, and thermodynamics are simultaneously considered. Under the assumption of a thermodynamic origin of gravity, we propose a general equation to describe the gravitational effect of quantum wave packets. In the classical limit, this equation agrees with Newton's law of gravitation. For quantum wave packets, however, it predicts a repulsive gravitational effect. We propose an experimental scheme using superfluid helium to test this repulsive gravitational effect. Our studies show that, with present technology such as superconducting gravimetry and cold atom interferometry, tests of the repulsive gravitational effect for superfluid helium are within experimental reach.

  8. Exciton-polariton localized wave packets in a microcavity

    NASA Astrophysics Data System (ADS)

    Voronych, Oksana; Buraczewski, Adam; Matuszewski, MichałÂ; Stobińska, Magdalena

    2016-06-01

    We investigate the possibility of creating X waves, or localized wave packets, in resonantly excited exciton-polariton superfluids. We demonstrate the existence of X-wave traveling solutions in the coupled exciton-photon system past the inflection point, where the effective mass of lower polaritons is negative in the direction perpendicular to the wave vector of the pumping beam. Contrary to the case of bright solitons, X waves do not require nonlinearity for sustaining their shape. Nevertheless, we show that nonlinearity is important for their dynamics, as it allows for their spontaneous formation from an initial Gaussian wave packet. Unique properties of exciton-polaritons may lead to applications of their X waves in long-distance signal propagation inside novel integrated optoelectronic circuits based on excitons.

  9. Nondispersive wave packets -- control through chaos

    NASA Astrophysics Data System (ADS)

    Buchleitner, Andreas

    2005-05-01

    Nondispersive wave packets were predicted to emerge in periodically driven Rydberg atoms a little more than 10 years ago [1], and have now been observed in the laboratory [2]. I shall illustrate how these robust, generic ``quantum particles'' and their relatives naturally emerge from the theory of chaotic quantum systems [3], and thus open new perspectives for robust quantum control in various experimental settings -- from one and two-electron [4] atoms under periodic or impulsive [5] driving to cold atoms in flashing periodic potentials, possibly amended by harmonic confinement [6]. Besides the fundamental underlying (nonlinear) resonance phenomena also some more subtle properties will be discussed, including open questions within the realm of spectral theory. *[1] A. Buchleitner, thèse de doctorat, Universit'e Paris 6 (1993); I. Bialynicki-Birula, M. Kalinski, and J. H. Eberly, Phys. Rev. Lett. 73, 1777 (1994); D. Delande and A. Buchleitner, Adv. At. Mol. Opt. Phys. 34, 85 (1994). *[2] H. Maeda and T. F. Gallagher, Phys. Rev. Lett. 92, 133004 (2004). *[3] A. Buchleitner, D. Delande, and J. Zakrzewski, Phys. Rep. 386, 409 (2002). *[4] J. Madroñero, PhD thesis, Ludwig-Maximilians-Universität München (2004), http://edoc.ub.uni-muenchen.de/archive/00002187. *[5] D.G. Arb'o et al., Phys. Rev. A 67, 63401 (2003). *[6] A.R.R. de Carvalho and A. Buchleitner, Phys. Rev. Lett. 93, 204101 (2004).

  10. Dynamics of Attosecond Electron Wave Packets

    NASA Astrophysics Data System (ADS)

    Mauritsson, Johan

    2005-05-01

    We present results from some of the first experimental studies of attosecond electron wave packets created via the absorption of ultrashort extreme ultraviolet (XUV) light pulses [1]. The pulses, made via high harmonic generation, form an attosecond pulse train (APT) whose properties we can manipulate by a combination of spatial and spectral filtering. For instance, we show that on-target attosecond pulses of 170 as duration, which is close to the single cycle limit, can be produced [2]. The electron wave packets created when such an APT is used to ionize an atom are different from the tunneling wave packets familiar from strong field ionization. We show how to measure the dynamics of these wave packets in a strong infrared (IR) field, where the absorption of energy above the ionization threshold is found to depend strongly on the APT-IR delay [3]. We also demonstrate that altering the properties of the initial electron wave packet by manipulating the APT changes the subsequent continuum electron dynamics. Finally, we show how the phase of a longer, femtosecond electron wave packet can be modulated by a moderately strong IR pulse with duration comparable to or shorter than that of the electron wave packet. This experiment reveals how the normal ponderomotive shift of an XUV ionization event is modified when the IR pulse is shorter than the XUV pulse.[1] The experiments were done at Lund Institute of Technology, Sweden.[2] R. López-Martens, et al., Phys. Rev. Lett. 94, 033001 (2005)[3] P. Johnsson, et al., submitted to Phys. Rev. Lett.

  11. Trajectory description of the quantum-classical transition for wave packet interference

    NASA Astrophysics Data System (ADS)

    Chou, Chia-Chun

    2016-08-01

    The quantum-classical transition for wave packet interference is investigated using a hydrodynamic description. A nonlinear quantum-classical transition equation is obtained by introducing a degree of quantumness ranging from zero to one into the classical time-dependent Schrödinger equation. This equation provides a continuous description for the transition process of physical systems from purely quantum to purely classical regimes. In this study, the transition trajectory formalism is developed to provide a hydrodynamic description for the quantum-classical transition. The flow momentum of transition trajectories is defined by the gradient of the action function in the transition wave function and these trajectories follow the main features of the evolving probability density. Then, the transition trajectory formalism is employed to analyze the quantum-classical transition of wave packet interference. For the collision-like wave packet interference where the propagation velocity is faster than the spreading speed of the wave packet, the interference process remains collision-like for all the degree of quantumness. However, the interference features demonstrated by transition trajectories gradually disappear when the degree of quantumness approaches zero. For the diffraction-like wave packet interference, the interference process changes continuously from a diffraction-like to collision-like case when the degree of quantumness gradually decreases. This study provides an insightful trajectory interpretation for the quantum-classical transition of wave packet interference.

  12. Test particle simulation study of whistler wave packets observed near Comet Giacobini-Zinner

    NASA Technical Reports Server (NTRS)

    Kaya, N.; Matsumoto, H.; Tsurutani, B. T.

    1989-01-01

    Nonlinear interactions of water group ions with large-amplitude whistler wave packets detected at the leading edge of steepened magnetosonic waves observed near Comet Giacobini-Zinner (GZ) are studied using test particle simulations of water-ion interactions with a model wave based on GZ data. Some of the water ions are found to be decelerated in the steepened portion of the magnetosonic wave to the resonance velocity with the whistler wave packets. Through resonance and related nonlinear interaction with the large-amplitude whistler waves, the water ions become trapped by the packet. An energy balance calculation demonstrates that the trapped ions lose their kinetic energy during the trapped motion in the packet. Thus, the nonlinear trapping motion in the wave structure leads to effective energy transfer from the water group ions to the whistler wave packets in the leading edge of the steepened MHD waves.

  13. Test particle simulation study of whistler wave packets observed near comet Giacobini-Zinner

    SciTech Connect

    Kaya, N. ); Matsumoto, H.; Tsurutani, B.T. California Institute of Technology, Pasadena )

    1989-01-01

    In order to study nonlinear interactions of water group ions with large amplitude whistler wave packets detected at the leading edge of steepened magnetosonic waves observed near comet Giacobini-Zinner, the authors carried out test particle simulations of water ion interactions with a model wave based on the G-Z data. As the model wave, they adopted a linearly polarized magnetosonic (MS) wave as the trailing portion of the wave, and circularly polarized whistler waves in the leading edge of the wave. Both the MS and whistler waves are a priori assumed to have large amplitudes. They found that some of the water ions are decelerated in the steepened portion of the magnetosonic wave to the resonance velocity with the whistler wave packets. Through resonance and related nonlinear interaction with the large amplitude whistler waves, the water ions become trapped by the whistler wave packet. An energy balance calculation demonstrates that the trapped ions do lose their kinetic energy during the trapped motion in the whistler wave packet. It is thus demonstrated that the nonlinear trapping motion in the wave structure leads to the effective energy transfer from the water group ions to the whistler wave packets in the leading edge of the steepened MHD waves.

  14. Momentum Imaging of Electron Wave Packet Interference

    NASA Astrophysics Data System (ADS)

    Liu, Aihua; He, Feng; Thumm, Uwe

    2010-03-01

    The recent experiment by Gopal, et al.[Phys. Rev. Lett. 103, 053001 (2009) ] detects intriguing interference patterns in the single ionization of helium by few-cycle, phase-stabilized IR laser pulses, which Gopal, et al. interpret in terms of the coherent emission of distinct photoelectron wave packets within one IR cycle. By numerically solving the time-dependent Schrödinger equation for the photoionization of helium within a single active electron model, we find interference fringes in the photoelectron momentum distribution that cannot be explained as above-threshold ionization peaks. We are in the process of analyzing these oscillations in the momentum-differential electron yield in terms of interfering photoelectron wave packets.

  15. Teleportation of nonclassical wave packets of light.

    PubMed

    Lee, Noriyuki; Benichi, Hugo; Takeno, Yuishi; Takeda, Shuntaro; Webb, James; Huntington, Elanor; Furusawa, Akira

    2011-04-15

    We report on the experimental quantum teleportation of strongly nonclassical wave packets of light. To perform this full quantum operation while preserving and retrieving the fragile nonclassicality of the input state, we have developed a broadband, zero-dispersion teleportation apparatus that works in conjunction with time-resolved state preparation equipment. Our approach brings within experimental reach a whole new set of hybrid protocols involving discrete- and continuous-variable techniques in quantum information processing for optical sciences. PMID:21493853

  16. Pressure fluctuations beneath turbulent spots and instability wave packets in a hypersonic boundary layer.

    SciTech Connect

    Beresh, Steven Jay; Casper, Katya M.; Schneider, Steven P.

    2010-12-01

    The development of turbulent spots in a hypersonic boundary layer was studied on the nozzle wall of the Boeing/AFOSR Mach-6 Quiet Tunnel. Under quiet flow conditions, the nozzle wall boundary layer remains laminar and grows very thick over the long nozzle length. This allows the development of large turbulent spots that can be readily measured with pressure transducers. Measurements of naturally occurring wave packets and developing turbulent spots were made. The peak frequencies of these natural wave packets were in agreement with second-mode computations. For a controlled study, the breakdown of disturbances created by spark and glow perturbations were studied at similar freestream conditions. The spark perturbations were the most effective at creating large wave packets that broke down into turbulent spots. The flow disturbances created by the controlled perturbations were analyzed to obtain amplitude criteria for nonlinearity and breakdown as well as the convection velocities of the turbulent spots. Disturbances first grew into linear instability waves and then quickly became nonlinear. Throughout the nonlinear growth of the wave packets, large harmonics are visible in the power spectra. As breakdown begins, the peak amplitudes of the instability waves and harmonics decrease into the rising broad-band frequencies. Instability waves are still visible on either side of the growing turbulent spots during this breakdown process.

  17. Spreading of atomic wave packets and semiclassical chaos

    NASA Astrophysics Data System (ADS)

    Argonov, V. Yu.

    2010-12-01

    The correspondence between the statistical properties of the evolution of a quantum system and Lyapunov instability and the chaos of its semiclassical analog has been demonstrated. The results of the analyses of atomic motion in a laser field in the semiclassical approximation (dynamics is described by several nonlinear equations) and without this approximation (dynamics is described by an infinite system of linear equations) are compared. In the ranges of the parameters for which the semiclassical dynamics of point-like atoms is unstable, the fast "spreading" of quantized wave packets in the momentum space is observed. Thus, deterministic chaos "imitates" the statistics of the quantum nondeterministic effects, although the semiclassical and quantum solutions are fundamentally different.

  18. Spreading of atomic wave packets and semiclassical chaos

    NASA Astrophysics Data System (ADS)

    Argonov, V. Yu.

    2009-12-01

    The correspondence between the statistical properties of the evolution of a quantum system and Lyapunov instability and the chaos of its semiclassical analog has been demonstrated. The results of the analyses of atomic motion in a laser field in the semiclassical approximation (dynamics is described by several nonlinear equations) and without this approximation (dynamics is described by an infinite system of linear equations) are compared. In the ranges of the parameters for which the semiclassical dynamics of point-like atoms is unstable, the fast “spreading” of quantized wave packets in the momentum space is observed. Thus, deterministic chaos “imitates” the statistics of the quantum nondeterministic effects, although the semiclassical and quantum solutions are fundamentally different.

  19. Propagation and breathing of matter-wave-packet trains

    SciTech Connect

    Hai Wenhua; Chong Guishu; Lee, Chaohong

    2004-11-01

    We find a set of different orthonormalized states of a nonstationary harmonic oscillator and use them to expand the solution of the Gross-Pitaevskii equation with harmonic potential. The expansion series describes wave-packet trains of a Bose-Einstein condensate, which may be induced initially by the modulational instability. The center of any wave-packet train oscillates like a classical harmonic oscillator of frequency {omega}. The width and height of the wave packet and the distance between two wave packets change simultaneously like an array of breathers with frequency 2{omega}. We demonstrate analytically and numerically that for a set of suitable parameters the wave-packet trains can be more exactly fitted to the matter-wave soliton trains observed by Strecker et al. and reported in Nature (London) 417, 150 (2002)

  20. Nondiffracting accelerating wave packets of Maxwell's equations.

    PubMed

    Kaminer, Ido; Bekenstein, Rivka; Nemirovsky, Jonathan; Segev, Mordechai

    2012-04-20

    We present the nondiffracting spatially accelerating solutions of the Maxwell equations. Such beams accelerate in a circular trajectory, thus generalizing the concept of Airy beams to the full domain of the wave equation. For both TE and TM polarizations, the beams exhibit shape-preserving bending which can have subwavelength features, and the Poynting vector of the main lobe displays a turn of more than 90°. We show that these accelerating beams are self-healing, analyze their properties, and find the new class of accelerating breathers: self-bending beams of periodically oscillating shapes. Finally, we emphasize that in their scalar form, these beams are the exact solutions for nondispersive accelerating wave packets of the most common wave equation describing time-harmonic waves. As such, this work has profound implications to many linear wave systems in nature, ranging from acoustic and elastic waves to surface waves in fluids and membranes. PMID:22680719

  1. Wave packets, transients, and numerical relativity

    NASA Astrophysics Data System (ADS)

    O'Shaughnessy, Richard

    2003-04-01

    Many in the numerical relativity community (e.g. Alcubierre et al (2000), Yoneda and Shinkai) have conjectured that formulations of relativity in which N fields propagate relative to coordinates will generally be more stable than formulations with M≤ N fields propagate. Loosely, errors can propagate away more effectively if more fields propagate. For first-order symmetric hyperbolic linear systems, we demonstrate (by way of explicit wave-packet solutions) that indeed most short-scale errors propagate away before growing to large magnitude. We also demonstrate that, for systems with long-lived characteristics (e.g. with horizons and physical characteristic speeds), the potential exists for unbounded growth of small errors, in a manner that could conceivably plague numerial evolutions. We discuss in particular the growth of transient errors in simulations of a Schwarzchild hole in Penelve-Gullstrand coordinates using the equations of Kidder, Scheel, and Teukolsky.

  2. Stability and evolution of wave packets in strongly coupled degenerate plasmas.

    PubMed

    Misra, A P; Shukla, P K

    2012-02-01

    We study the nonlinear propagation of electrostatic wave packets in a collisional plasma composed of strongly coupled ions and relativistically degenerate electrons. The equilibrium of ions is maintained by an effective temperature associated with their strong coupling, whereas that of electrons is provided by the relativistic degeneracy pressure. Using a multiple-scale technique, a (3 + 1)-dimensional coupled set of nonlinear Schrödinger-like equations with nonlocal nonlinearity is derived from a generalized viscoelastic hydrodynamic model. These coupled equations, which govern the dynamics of wave packets, are used to study the oblique modulational instability of a Stoke's wave train to a small plane-wave perturbation. We show that the wave packets, though stable to the parallel modulation, become unstable against oblique modulations. In contrast to the long-wavelength carrier modes, the wave packets with short wavelengths are shown to be stable in the weakly relativistic case, whereas they can be stable or unstable in the ultrarelativistic limit. Numerical simulation of the coupled equations reveals that a steady-state solution of the wave amplitude exists together with the formation of a localized structure in (2 + 1) dimensions. However, in the (3 + 1)-dimensional evolution, a Gaussian wave beam self-focuses after interaction and blows up in a finite time. The latter is, however, arrested when the dispersion predominates over the nonlinearities. This occurs when the Coulomb coupling strength is higher or a choice of obliqueness of modulation, or a wavelength of excitation is different. Possible application of our results to the interior as well as in an outer mantle of white dwarfs are discussed. PMID:22463339

  3. Observation of Quantum Interference between Separated Mechanical Oscillator Wave Packets.

    PubMed

    Kienzler, D; Flühmann, C; Negnevitsky, V; Lo, H-Y; Marinelli, M; Nadlinger, D; Home, J P

    2016-04-01

    We directly observe the quantum interference between two well-separated trapped-ion mechanical oscillator wave packets. The superposed state is created from a spin-motion entangled state using a heralded measurement. Wave packet interference is observed through the energy eigenstate populations. We reconstruct the Wigner function of these states by introducing probe Hamiltonians which measure Fock state populations in displaced and squeezed bases. Squeezed-basis measurements with 8 dB squeezing allow the measurement of interference for Δα=15.6, corresponding to a distance of 240 nm between the two superposed wave packets. PMID:27104686

  4. Observation of Quantum Interference between Separated Mechanical Oscillator Wave Packets

    NASA Astrophysics Data System (ADS)

    Kienzler, D.; Flühmann, C.; Negnevitsky, V.; Lo, H.-Y.; Marinelli, M.; Nadlinger, D.; Home, J. P.

    2016-04-01

    We directly observe the quantum interference between two well-separated trapped-ion mechanical oscillator wave packets. The superposed state is created from a spin-motion entangled state using a heralded measurement. Wave packet interference is observed through the energy eigenstate populations. We reconstruct the Wigner function of these states by introducing probe Hamiltonians which measure Fock state populations in displaced and squeezed bases. Squeezed-basis measurements with 8 dB squeezing allow the measurement of interference for Δ α =15.6 , corresponding to a distance of 240 nm between the two superposed wave packets.

  5. Wave-packet formation at the zero-dispersion point in the Gardner-Ostrovsky equation.

    PubMed

    Whitfield, A J; Johnson, E R

    2015-05-01

    The long-time effect of weak rotation on an internal solitary wave is the decay into inertia-gravity waves and the eventual emergence of a coherent, steadily propagating, nonlinear wave packet. There is currently no entirely satisfactory explanation as to why these wave packets form. Here the initial value problem is considered within the context of the Gardner-Ostrovsky, or rotation-modified extended Korteweg-de Vries, equation. The linear Gardner-Ostrovsky equation has maximum group velocity at a critical wave number, often called the zero-dispersion point. It is found here that a nonlinear splitting of the wave-number spectrum at the zero-dispersion point, where energy is shifted into the modulationally unstable regime of the Gardner-Ostrovsky equation, is responsible for the wave-packet formation. Numerical comparisons of the decay of a solitary wave in the Gardner-Ostrovsky equation and a derived nonlinear Schrödinger equation at the zero-dispersion point are used to confirm the spectral splitting. PMID:26066112

  6. Analytic approach to the wave packet formalism in oscillation phenomena

    SciTech Connect

    Bernardini, A.E.; Leo, S. de

    2004-09-01

    We introduce an approximation scheme to perform an analytic study of the oscillation phenomena in a pedagogical and comprehensive way. By using Gaussian wave packets, we show that the oscillation is bounded by a time-dependent vanishing function which characterizes the slippage between the mass-eigenstate wave packets. We also demonstrate that the wave packet spreading represents a secondary effect which plays a significant role only in the nonrelativistic limit. In our analysis, we note the presence of a new time-dependent phase and calculate how this additional term modifies the oscillating character of the flavor conversion formula. Finally, by considering box and sine wave packets we study how the choice of different functions to describe the particle localization changes the oscillation probability.

  7. Observation of Nonspreading Wave Packets in an Imaginary Potential

    SciTech Connect

    Stuetzle, R.; Goebel, M.C.; Hoerner, Th.; Kierig, E.; Mourachko, I.; Oberthaler, M.K.; Efremov, M.A.; Fedorov, M.V.; Yakovlev, V.P.; Leeuwen, K.A.H. van; Schleich, W.P.

    2005-09-09

    We propose and experimentally demonstrate a method to prepare a nonspreading atomic wave packet. Our technique relies on a spatially modulated absorption constantly chiseling away from an initially broad de Broglie wave. The resulting contraction is balanced by dispersion due to Heisenberg's uncertainty principle. This quantum evolution results in the formation of a nonspreading wave packet of Gaussian form with a spatially quadratic phase. Experimentally, we confirm these predictions by observing the evolution of the momentum distribution. Moreover, by employing interferometric techniques, we measure the predicted quadratic phase across the wave packet. Nonspreading wave packets of this kind also exist in two space dimensions and we can control their amplitude and phase using optical elements.

  8. Localization of wave packets in one-dimensional random potentials

    NASA Astrophysics Data System (ADS)

    Valdes, Juan Pablo Ramírez; Wellens, Thomas

    2016-06-01

    We study the expansion of an initially strongly confined wave packet in a one-dimensional weak random potential with short correlation length. At long times, the expansion of the wave packet comes to a halt due to destructive interferences leading to Anderson localization. We develop an analytical description for the disorder-averaged localized density profile. For this purpose, we employ the diagrammatic method of Berezinskii which we extend to the case of wave packets, present an analytical expression of the Lyapunov exponent which is valid for small as well as for high energies, and, finally, develop a self-consistent Born approximation in order to analytically calculate the energy distribution of our wave packet. By comparison with numerical simulations, we show that our theory describes well the complete localized density profile, not only in the tails but also in the center.

  9. Stochastic Motion of Relativistic Particles in the Field of a Wide Wave Packet

    NASA Astrophysics Data System (ADS)

    Nagornykh, E.; Tel'nikhin, A.

    2003-06-01

    Stochastic motion of relativistic particles in the field of a wave packet propagating under an angle to the external magnetic field are investigated. The interplay of the dynamical and statistical aspects of the behavior of the relativistic particle-potential wave packet system is considered. Dynamics of this system are described by nonlinear mapping and corresponding Fokker-Planck-Kolmogorov equation in phase space possesses canonical Hamiltonian structure. The following general problems of stochastic motion are disscussed: local instability and the Lyapunov exponents and the Kolmogorov entropy; a fractal structures and its dimension; bifurcations of a vector fields and the boundaries of the region of dynamical chaos. The results of numerical simulation are presented. A possible astrophysical application of the results obtained is discussed.

  10. Direct observation of an attosecond electron wave packet in a nitrogen molecule

    PubMed Central

    Okino, Tomoya; Furukawa, Yusuke; Nabekawa, Yasuo; Miyabe, Shungo; Amani Eilanlou, A.; Takahashi, Eiji J.; Yamanouchi, Kaoru; Midorikawa, Katsumi

    2015-01-01

    Capturing electron motion in a molecule is the basis of understanding or steering chemical reactions. Nonlinear Fourier transform spectroscopy using an attosecond-pump/attosecond-probe technique is used to observe an attosecond electron wave packet in a nitrogen molecule in real time. The 500-as electronic motion between two bound electronic states in a nitrogen molecule is captured by measuring the fragment ions with the same kinetic energy generated in sequential two-photon dissociative ionization processes. The temporal evolution of electronic coherence originating from various electronic states is visualized via the fragment ions appearing after irradiation of the probe pulse. This observation of an attosecond molecular electron wave packet is a critical step in understanding coupled nuclear and electron motion in polyatomic and biological molecules to explore attochemistry. PMID:26601262

  11. Wave modulation: the geometry, kinematics, and dynamics of surface-wave packets

    NASA Astrophysics Data System (ADS)

    Pizzo, Nicholas; Melville, W. Kendall

    2015-11-01

    We derive moment evolution equations of the modified nonlinear Schrodinger equation (MNLSE) with application to interpreting the geometry, kinematics and dynamics of focusing deep-water wave packets. Our theory predicts modifications to the group velocity and associates wave packet convergence with the breakdown of equipartition between kinetic and potential energy. The evolution of the first moment of the energy density yields a natural way to interpret the concept of group velocity for these compact wave groups, predicting a velocity increase as the packet focuses, and is found to be up to 10% larger than that predicted by linear theory, consistent with laboratory observations. The second moment yields a virial theorem, associating energy convergence with deviations from equipartition. The derivation of these moment equations relies crucially on the variational structure of the spatial version of the MNLSE, and the subsequent derivation of three conservations laws. These predictions are then examined numerically for focusing wave packets governed by both the MNLSE as well as the full potential flow equations, and the results are discussed in the context of existing theoretical, numerical and laboratory studies.

  12. Sinusoidal nonlinearity in wavelength-sweeping interferometry

    SciTech Connect

    Perret, Luc; Pfeiffer, Pierre

    2007-11-20

    We report the influence of the nonlinearities in the wavelength-sweeping speed on the resulting interferometric signals in an absolute distance interferometer. The sweeping signal is launched in the reference and target interferometers from an external cavity laser source. The experimental results demonstrate a good resolution in spite of the presence of nonlinearities in the wavelength sweep. These nonlinearities can be modeled by a sum of sinusoids. A simulation is then implemented to analyze the influence of their parameters. It shows that a sinusoidal nonlinearity is robust enough to give a good final measurement uncertainty through a Fourier transform technique. It can be concluded that an optimal value of frequency and amplitude exists in the case of a sinusoidal nonlinearity.

  13. Sinusoidal nonlinearity in wavelength-sweeping interferometry.

    PubMed

    Perret, Luc; Pfeiffer, Pierre

    2007-11-20

    We report the influence of the nonlinearities in the wavelength-sweeping speed on the resulting interferometric signals in an absolute distance interferometer. The sweeping signal is launched in the reference and target interferometers from an external cavity laser source. The experimental results demonstrate a good resolution in spite of the presence of nonlinearities in the wavelength sweep. These nonlinearities can be modeled by a sum of sinusoids. A simulation is then implemented to analyze the influence of their parameters. It shows that a sinusoidal nonlinearity is robust enough to give a good final measurement uncertainty through a Fourier transform technique. It can be concluded that an optimal value of frequency and amplitude exists in the case of a sinusoidal nonlinearity. PMID:18026546

  14. Pressure fluctuations beneath instability wave packets and turbulent spots in a hypersonic boundary layer

    NASA Astrophysics Data System (ADS)

    Casper, Katya M.

    During atmospheric reentry, hypersonic vehicles are subjected to high levels of boundary-layer pressure fluctuations that cause vibration of internal components. Current models are not adequate to predict these fluctuations. A more physics-based approach can be obtained by using a turbulent-spot model of transition. In order to gain a better understanding of the pressure-fluctuation field and the growth of turbulent spots in a hypersonic boundary layer, the development of disturbances was studied on the nozzle wall of the Boeing/AFOSR Mach-6 Quiet Tunnel. Under quiet flow conditions, the nozzle wall boundary layer remains laminar and grows very thick over the long nozzle length. This allows the development of large disturbances that can be well-resolved with high-frequency pressure transducers. For a controlled study, disturbances were created by pulsed glow perturbations and studied at various freestream conditions. Both the centerline and the spanwise distribution of pressure fluctuations were measured as boundary-layer disturbances grew from linear instability wave packets into turbulent spots. A disturbance first grows into a linear instability wave packet and then quickly becomes nonlinear. At this point, the wave packet is still concentrated near the disturbance centerline, but weaker disturbances are seen spreading from the center. Throughout the nonlinear growth of the wave packets, large harmonics are visible in the power spectra. Breakdown to turbulence begins in the core of the wave packets where the wave amplitudes are largest. As breakdown begins, the peak amplitudes of the instability waves and harmonics decrease into the rising broadband frequencies. Second-mode waves are still evident in front of and behind the breakdown point and can be seen propagating in the spanwise direction at a spreading angle. The turbulent core grows downstream, resulting in a turbulent spot with a typical arrowhead shape. However, the spot is not merely a localized patch

  15. Two Color Interferometry with Nonlinear Refractive Properties

    NASA Technical Reports Server (NTRS)

    Vikram, Chandra S.; Witherow, William K.

    2002-01-01

    Using nonlinear refractive properties of salt-water solution at two wavelengths, numerical analysis has been performed to extract temperature and concentration from virtual interferometric fringe data. The theoretical study, using a commercially available equation solving tool, starts with critical fringe counting needs and the role of nonlinear refractive properties in such measurements. Finally, methodology of the analysis, developed codes, and fringe counting accuracy needs are described in detail.

  16. Attosecond Electron Wave Packet Dynamics in Strong Laser Fields

    SciTech Connect

    Johnsson, P.; Remetter, T.; Varju, K.; L'Huillier, A.; Lopez-Martens, R.; Valentin, C.; Balcou, Ph.; Kazamias, S.; Mauritsson, J.; Gaarde, M. B.; Schafer, K. J.; Mairesse, Y.; Wabnitz, H.; Salieres, P.

    2005-07-01

    We use a train of sub-200 attosecond extreme ultraviolet (XUV) pulses with energies just above the ionization threshold in argon to create a train of temporally localized electron wave packets. We study the energy transfer from a strong infrared (IR) laser field to the ionized electrons as a function of the delay between the XUV and IR fields. When the wave packets are born at the zero crossings of the IR field, a significant amount of energy ({approx}20 eV) is transferred from the field to the electrons. This results in dramatically enhanced above-threshold ionization in conditions where the IR field alone does not induce any significant ionization. Because both the energy and duration of the wave packets can be varied independently of the IR laser, they are valuable tools for studying and controlling strong-field processes.

  17. Semiclassical Dynamics of Electron Wave Packet States with Phase Vortices

    SciTech Connect

    Bliokh, Konstantin Yu.; Bliokh, Yury P.; Savel'ev, Sergey; Nori, Franco

    2007-11-09

    We consider semiclassical higher-order wave packet solutions of the Schroedinger equation with phase vortices. The vortex line is aligned with the propagation direction, and the wave packet carries a well-defined orbital angular momentum (OAM) ({Dirac_h}/2{pi})l (l is the vortex strength) along its main linear momentum. The probability current coils around the momentum in such OAM states of electrons. In an electric field, these states evolve like massless particles with spin l. The magnetic-monopole Berry curvature appears in momentum space, which results in a spin-orbit-type interaction and a Berry/Magnus transverse force acting on the wave packet. This brings about the OAM Hall effect. In a magnetic field, there is a Zeeman interaction, which, can lead to more complicated dynamics.

  18. Chiral wave-packet scattering in Weyl semimetals

    NASA Astrophysics Data System (ADS)

    Jiang, Qing-Dong; Jiang, Hua; Liu, Haiwen; Sun, Qing-Feng; Xie, X. C.

    2016-05-01

    In quantum mechanics, a particle is best described by the wave packet instead of the plane wave. Here, we study the wave-packet scattering problem in Weyl semimetals with the low-energy Weyl fermions of different chiralities. Our results show that the wave packet acquires a chirality-protected shift in the single-impurity scattering process. More importantly, the chirality-protected shift can lead to an anomalous scattering probability, and thus affects the transport properties in Weyl semimetals. We find that the ratio between the transport lifetime and the quantum lifetime increases sharply when the Fermi energy approaches the Weyl nodes, providing an explanation of the experimentally observed ultrahigh mobility in topological (Weyl or Dirac) semimetals.

  19. Wave packet propagation across barriers by semiclassical initial value methods

    NASA Astrophysics Data System (ADS)

    Petersen, Jakob; Kay, Kenneth G.

    2015-07-01

    Semiclassical initial value representation (IVR) formulas for the propagator have difficulty describing tunneling through barriers. A key reason is that these formulas do not automatically reduce, in the classical limit, to the version of the Van Vleck-Gutzwiller (VVG) propagator required to treat barrier tunneling, which involves trajectories that have complex initial conditions and that follow paths in complex time. In this work, a simple IVR expression, that has the correct tunneling form in the classical limit, is derived for the propagator in the case of one-dimensional barrier transmission. Similarly, an IVR formula, that reduces to the Generalized Gaussian Wave Packet Dynamics (GGWPD) expression [D. Huber, E. J. Heller, and R. Littlejohn, J. Chem. Phys. 89, 2003 (1988)] in the classical limit, is derived for the transmitted wave packet. Uniform semiclassical versions of the IVR formulas are presented and simplified expressions in terms of real trajectories and WKB penetration factors are described. Numerical tests show that the uniform IVR treatment gives good results for wave packet transmission through the Eckart and Gaussian barriers in all cases examined. In contrast, even when applied with the proper complex trajectories, the VVG and GGWPD treatments are inaccurate when the mean energy of the wave packet is near the classical transmission threshold. The IVR expressions for the propagator and wave packet are cast as contour integrals in the complex space of initial conditions and these are generalized to potentially allow treatment of a larger variety of systems. A steepest descent analysis of the contour integral formula for the wave packet in the present cases confirms its relationship to the GGWPD method, verifies its semiclassical validity, and explains results of numerical calculations.

  20. Coda wave interferometry for estimating nonlinear behavior in seismic velocity.

    PubMed

    Snieder, Roel; Grêt, Alexandre; Douma, Huub; Scales, John

    2002-03-22

    In coda wave interferometry, one records multiply scattered waves at a limited number of receivers to infer changes in the medium over time. With this technique, we have determined the nonlinear dependence of the seismic velocity in granite on temperature and the associated acoustic emissions. This technique can be used in warning mode, to detect the presence of temporal changes in the medium, or in diagnostic mode, where the temporal change in the medium is quantified. PMID:11910107

  1. Short-time Chebyshev wave packet method for molecular photoionization

    NASA Astrophysics Data System (ADS)

    Sun, Zhaopeng; Zheng, Yujun

    2016-08-01

    In this letter we present the extended usage of short-time Chebyshev wave packet method in the laser induced molecular photoionization dynamics. In our extension, the polynomial expansion of the exponential in the time evolution operator, the Hamiltonian operator can act on the wave packet directly which neatly avoids the matrix diagonalization. This propagation scheme is of obvious advantages when the dynamical system has large Hamiltonian matrix. Computational simulations are performed for the calculation of photoelectronic distributions from intense short pulse ionization of K2 and NaI which represent the Born-Oppenheimer (BO) model and Non-BO one, respectively.

  2. Wave packet dynamics under effect of a pulsed electric field

    NASA Astrophysics Data System (ADS)

    da Silva, A. R. C. B.; de Moura, F. A. B. F.; Dias, W. S.

    2016-06-01

    We studied the dynamics of an electron in a crystalline one-dimensional model under effect of a time-dependent Gaussian field. The time evolution of an initially Gaussian wave packet it was obtained through the numerical solution of the time-dependent Schrödinger equation. Our analysis consists of computing the electronic centroid as well as the mean square displacement. We observe that the electrical pulse is able to promote a special kind of displacement along the chain. We demonstrated a direct relation between the group velocity of the wave packet and the applied electrical pulses. We compare those numerical calculations with a semi-classical approach.

  3. Gabor Wave Packet Method to Solve Plasma Wave Equations

    SciTech Connect

    A. Pletzer; C.K. Phillips; D.N. Smithe

    2003-06-18

    A numerical method for solving plasma wave equations arising in the context of mode conversion between the fast magnetosonic and the slow (e.g ion Bernstein) wave is presented. The numerical algorithm relies on the expansion of the solution in Gaussian wave packets known as Gabor functions, which have good resolution properties in both real and Fourier space. The wave packets are ideally suited to capture both the large and small wavelength features that characterize mode conversion problems. The accuracy of the scheme is compared with a standard finite element approach.

  4. Symmetry and conservation laws in semiclassical wave packet dynamics

    SciTech Connect

    Ohsawa, Tomoki

    2015-03-15

    We formulate symmetries in semiclassical Gaussian wave packet dynamics and find the corresponding conserved quantities, particularly the semiclassical angular momentum, via Noether’s theorem. We consider two slightly different formulations of Gaussian wave packet dynamics; one is based on earlier works of Heller and Hagedorn and the other based on the symplectic-geometric approach by Lubich and others. In either case, we reveal the symplectic and Hamiltonian nature of the dynamics and formulate natural symmetry group actions in the setting to derive the corresponding conserved quantities (momentum maps). The semiclassical angular momentum inherits the essential properties of the classical angular momentum as well as naturally corresponds to the quantum picture.

  5. Perfect wave-packet splitting and reconstruction in a one-dimensional lattice

    NASA Astrophysics Data System (ADS)

    Banchi, Leonardo; Compagno, Enrico; Bose, Sougato

    2015-05-01

    Particle delocalization is a common feature of quantum random walks in arbitrary lattices. However, in the typical scenario a particle spreads over multiple sites and its evolution is not directly useful for controlled quantum interferometry, as may be required for technological applications. In this paper we devise a strategy to perfectly split the wave packet of an incoming particle into two components, each propagating in opposite directions, which reconstruct the shape of the initial wavefunction after a particular time t*. Therefore, a particle in a δ -like initial state becomes exactly delocalized between two distant sites after t*. We find the mathematical conditions to achieve the perfect splitting, which are satisfied by viable example Hamiltonians with static site-dependent interaction strengths. Our results pave the way for the generation of peculiar many-body interference patterns in a many-site atomic chain (such as the Hanbury Brown and Twiss and quantum Talbot effects) as well as for the distribution of entanglement between remote sites. Thus, as for the case of perfect state transfer, the perfect wave-packet splitting can be a new tool for varied applications.

  6. Asymmetric Acoustic Propagation of Wave Packets Via the Self-Demodulation Effect.

    PubMed

    Devaux, Thibaut; Tournat, Vincent; Richoux, Olivier; Pagneux, Vincent

    2015-12-01

    This Letter presents the experimental characterization of nonreciprocal elastic wave transmission in a single-mode elastic waveguide. This asymmetric system is obtained by coupling a selection layer with a conversion layer: the selection component is provided by a phononic crystal, while the conversion is achieved by a nonlinear self-demodulation effect in a 3D unconsolidated granular medium. A quantitative experimental study of this acoustic rectifier indicates a high rectifying ratio, up to 10^{6}, with wide band (10 kHz) and an audible effect. Moreover, this system allows for wave-packet rectification and extends the future applications of asymmetric systems. PMID:26684119

  7. Asymmetric Acoustic Propagation of Wave Packets Via the Self-Demodulation Effect

    NASA Astrophysics Data System (ADS)

    Devaux, Thibaut; Tournat, Vincent; Richoux, Olivier; Pagneux, Vincent

    2015-12-01

    This Letter presents the experimental characterization of nonreciprocal elastic wave transmission in a single-mode elastic waveguide. This asymmetric system is obtained by coupling a selection layer with a conversion layer: the selection component is provided by a phononic crystal, while the conversion is achieved by a nonlinear self-demodulation effect in a 3D unconsolidated granular medium. A quantitative experimental study of this acoustic rectifier indicates a high rectifying ratio, up to 1 06, with wide band (10 kHz) and an audible effect. Moreover, this system allows for wave-packet rectification and extends the future applications of asymmetric systems.

  8. Modulation instability of wave packets in a Gires-Tournois interferometer

    NASA Astrophysics Data System (ADS)

    Zolotovskii, I. O.; Lapin, V. A.; Sementsov, D. I.

    2016-07-01

    We study the specific features of the perturbation dynamics of a wave packet in a Gires-Tournois interferometer. We obtain a dispersion relationship that relates the perturbation parameters to the parameters of the structure and pump wave, the analytical expressions for the gain increment of a harmonic perturbation and other important characteristics that determine the dynamics of the modulation instability of the reflected wave. Based on numerical simulation, we plot the dependences of the dispersion and nonlinearity parameters and the gain increment on the spacing between the interferometer mirrors, the angle of incidence of the radiation onto the mirrors, and the radiation intensity.

  9. Direct Harmonic Linear Navier-Stokes Methods for Efficient Simulation of Wave Packets

    NASA Technical Reports Server (NTRS)

    Streett, C. L.

    1998-01-01

    Wave packets produced by localized disturbances play an important role in transition in three-dimensional boundary layers, such as that on a swept wing. Starting with the receptivity process, we show the effects of wave-space energy distribution on the development of packets and other three-dimensional disturbance patterns. Nonlinearity in the receptivity process is specifically addressed, including demonstration of an effect which can enhance receptivity of traveling crossflow disturbances. An efficient spatial numerical simulation method is allowing most of the simulations presented to be carried out on a workstation.

  10. Wave packet motion in harmonic potential and computer visualization

    NASA Technical Reports Server (NTRS)

    Tsuru, Hideo; Kobayashi, Takeshi

    1993-01-01

    Wave packet motions of a single electron in harmonic potentials or a magnetic field are obtained analytically. The phase of the wave function which depends on both time and space is also presented explicitly. The probability density of the electron changes its width and central position periodically. These results are visualized using computer animation techniques.

  11. Resonance-assisted decay of nondispersive wave packets.

    PubMed

    Wimberger, Sandro; Schlagheck, Peter; Eltschka, Christopher; Buchleitner, Andreas

    2006-07-28

    We present a quantitative semiclassical theory for the decay of nondispersive electronic wave packets in driven, ionizing Rydberg systems. Statistically robust quantities are extracted combining resonance-assisted tunneling with subsequent transport across chaotic phase space and a final ionization step. PMID:16907569

  12. Nonlinear interferometry approach to photonic sequential logic

    NASA Astrophysics Data System (ADS)

    Mabuchi, Hideo

    2011-10-01

    Motivated by rapidly advancing capabilities for extensive nanoscale patterning of optical materials, I propose an approach to implementing photonic sequential logic that exploits circuit-scale phase coherence for efficient realizations of fundamental components such as a NAND-gate-with-fanout and a bistable latch. Kerr-nonlinear optical resonators are utilized in combination with interference effects to drive the binary logic. Quantum-optical input-output models are characterized numerically using design parameters that yield attojoule-scale energy separation between the latch states.

  13. Exploring multiple degrees of freedom in Rydberg wave packets

    NASA Astrophysics Data System (ADS)

    Wen, Haidan

    2006-12-01

    Recent advances in the study of Rydberg atoms have focused on the control, manipulation and detection of Rydberg wave packets using novel external fields such as half-cycle pulses. The radial degree of freedom has been controlled and used to process information encoded in Rydberg states. However, these previous experiments make use of only a single degree of freedom, restricting the potential of other degrees of freedom for quantum computing in Rydberg atoms. In this dissertation, we explore the control and detection of other degrees of freedom in an electron wave packet, such as the angular momentum quantum number ℓ, the magnetic quantum number m and the electron spin; so that the full range of quantum numbers can participate in information processing. We first propose an interferometric control of the population of angular momentum states using two time-delayed phase-locked ultrafast laser pulses. The population of arbitrary angular momentum states can be greatly enhanced by optimizing the time delay and the relative phases between two laser pulses. We then qualitatively measure the evolution of angular momentum components in Stark wave packets by a weak half-cycle pulse (HCP). This measurement utilizes a time-delayed HCP and is proved to be effective for detecting various aspects of wave packet dynamics, particularly, the evolution of non-stationary states. The technique relies on the fact that the HCP redistributes the eigenstate populations and induced the population variation which reflects the evolution of eigenstate phases. Finally, we find that the dynamics of m-states could be highly correlated with the internal degree of freedom of the electron, the spin. We study the effect of spin-orbit coupling on the wave packet dynamics and observe the angular precession of a Rydberg wave packet. The population redistribution from p to s states is highly sensitive to the polarization of the HCP and changes with the precession of the electron orbit. We obtain the

  14. Nonlinear interferometry with Bose-Einstein condensates

    SciTech Connect

    Tacla, Alexandre B.; Boixo, Sergio; Datta, Animesh; Shaji, Anil; Caves, Carlton M.

    2010-11-15

    We analyze a proposed experiment [Boixo et al., Phys. Rev. Lett. 101, 040403 (2008)] for achieving sensitivity scaling better than 1/N in a nonlinear Ramsey interferometer that uses a two-mode Bose-Einstein condensate (BEC) of N atoms. We present numerical simulations that confirm the analytical predictions for the effect of the spreading of the BEC ground-state wave function on the ideal 1/N{sup 3/2} scaling. Numerical integration of the coupled, time-dependent, two-mode Gross-Pitaevskii equations allows us to study the several simplifying assumptions made in the initial analytic study of the proposal and to explore when they can be justified. In particular, we find that the two modes share the same spatial wave function for a length of time that is sufficient to run the metrology scheme.

  15. Magnetic-Field Asymmetry of Electron Wave Packet Transmission in Bent Channels Capacitively Coupled to a Metal Gate

    NASA Astrophysics Data System (ADS)

    Kalina, R.; Szafran, B.; Bednarek, S.; Peeters, F. M.

    2009-02-01

    We study the electron wave packet moving through a bent channel. We demonstrate that the packet transmission probability becomes an asymmetric function of the magnetic field when the electron packet is capacitively coupled to a metal plate. The coupling occurs through a nonlinear potential which translates a different kinetics of the transport for opposite magnetic-field orientations into a different potential felt by the scattered electron.

  16. Stochastic acceleration of ions driven by Pc1 wave packets

    SciTech Connect

    Khazanov, G. V. Sibeck, D. G.; Tel'nikhin, A. A.; Kronberg, T. K.

    2015-07-15

    The stochastic motion of protons and He{sup +} ions driven by Pc1 wave packets is studied in the context of resonant particle heating. Resonant ion cyclotron heating typically occurs when wave powers exceed 10{sup −4} nT{sup 2}/Hz. Gyroresonance breaks the first adiabatic invariant and energizes keV ions. Cherenkov resonances with the electrostatic component of wave packets can also accelerate ions. The main effect of this interaction is to accelerate thermal protons to the local Alfven speed. The dependencies of observable quantities on the wave power and plasma parameters are determined, and estimates for the heating extent and rate of particle heating in these wave-particle interactions are shown to be in reasonable agreement with known empirical data.

  17. The Interference of the Dynamically Squeezed Vibrational Wave Packets

    NASA Technical Reports Server (NTRS)

    Vinogradov, An. V.; Janszky, J.; Kobayashi, T.

    1996-01-01

    An electronic excitation of a molecule by a sequence of two femtosecond phase-locked laser pulses is considered. In this case the interference between the vibrational wave packets induced by each of the subpulses within a single molecule takes place. It is shown that due to the dynamical squeezing effect of a molecular vibrational state the interference of the vibrational wave packets allows one to measure the duration of a femtosecond laser pulse. This can be achieved experimentally by measuring the dependence of the integral fluorescence of the excited molecule on the delay time between the subpulses. The interference can lead to a sharp peak (or to a down-fall) in that dependence, the width of which is equal to the duration of the laser pulse. It is shown that finite temperature of the medium is favorable for such an experiment.

  18. Wave packet dynamics in the optimal superadiabatic approximation

    NASA Astrophysics Data System (ADS)

    Betz, V.; Goddard, B. D.; Manthe, U.

    2016-06-01

    We explain the concept of superadiabatic representations and show how in the context of electronically non-adiabatic transitions they lead to an explicit formula that can be used to predict transitions at avoided crossings. Based on this formula, we present a simple method for computing wave packet dynamics across avoided crossings. Only knowledge of the adiabatic potential energy surfaces near the avoided crossing is required for the computation. In particular, this means that no diabatization procedure is necessary, the adiabatic electronic energies can be computed on the fly, and they only need to be computed to higher accuracy when an avoided crossing is detected. We test the quality of our method on the paradigmatic example of photo-dissociation of NaI, finding very good agreement with results of exact wave packet calculations.

  19. Spin-orbit states of neutron wave packets

    NASA Astrophysics Data System (ADS)

    Nsofini, Joachim; Sarenac, Dusan; Wood, Christopher J.; Cory, David G.; Arif, Muhammad; Clark, Charles W.; Huber, Michael G.; Pushin, Dmitry A.

    2016-07-01

    We propose a method to prepare an entangled spin-orbit state between the spin and the orbital angular momenta of a neutron wave packet. This spin-orbit state is created by passing neutrons through the center of a quadrupole magnetic field, which provides a coupling between the spin and orbital degrees of freedom. A Ramsey-fringe-type measurement is suggested as a means of verifying the spin-orbit correlations.

  20. Universal potential-barrier penetration by initially confined wave packets

    SciTech Connect

    Granot, Er'el; Marchewka, Avi

    2007-07-15

    The dynamics of an initially sharp-boundary wave packet in the presence of an arbitrary potential barrier is investigated. It is shown that the penetration through the barrier is universal in the sense that it depends only on the values of the wave function and its derivatives at the boundary. The dependence on the derivatives vanishes at long distances from the barrier, where the dynamics is governed solely by the initial value of the wave function at the boundary.

  1. Accelerating Airy-Gauss-Kummer localized wave packets

    NASA Astrophysics Data System (ADS)

    Zhong, Wei-Ping; Belić, Milivoj; Zhang, Yiqi; Huang, Tingwen

    2014-01-01

    A general approach to generating three-dimensional nondiffracting spatiotemporal solutions of the linear Schrödinger equation with an Airy-beam time-dependence is reported. A class of accelerating optical pulses with the structure of Airy-Gauss-Kummer vortex beams is obtained. Our results demonstrate that the optical field contributions to the Airy-Gauss-Kummer accelerating optical wave packets of the cylindrical symmetry can be characterized by the radial and angular mode numbers.

  2. Electronically nonadiabatic wave packet propagation using frozen Gaussian scattering.

    PubMed

    Kondorskiy, Alexey D; Nanbu, Shinkoh

    2015-09-21

    We present an approach, which allows to employ the adiabatic wave packet propagation technique and semiclassical theory to treat the nonadiabatic processes by using trajectory hopping. The approach developed generates a bunch of hopping trajectories and gives all additional information to incorporate the effect of nonadiabatic coupling into the wave packet dynamics. This provides an interface between a general adiabatic frozen Gaussian wave packet propagation method and the trajectory surface hopping technique. The basic idea suggested in [A. D. Kondorskiy and H. Nakamura, J. Chem. Phys. 120, 8937 (2004)] is revisited and complemented in the present work by the elaboration of efficient numerical algorithms. We combine our approach with the adiabatic Herman-Kluk frozen Gaussian approximation. The efficiency and accuracy of the resulting method is demonstrated by applying it to popular benchmark model systems including three Tully's models and 24D model of pyrazine. It is shown that photoabsorption spectrum is successfully reproduced by using a few hundreds of trajectories. We employ the compact finite difference Hessian update scheme to consider feasibility of the ab initio "on-the-fly" simulations. It is found that this technique allows us to obtain the reliable final results using several Hessian matrix calculations per trajectory. PMID:26395683

  3. Electronically nonadiabatic wave packet propagation using frozen Gaussian scattering

    NASA Astrophysics Data System (ADS)

    Kondorskiy, Alexey D.; Nanbu, Shinkoh

    2015-09-01

    We present an approach, which allows to employ the adiabatic wave packet propagation technique and semiclassical theory to treat the nonadiabatic processes by using trajectory hopping. The approach developed generates a bunch of hopping trajectories and gives all additional information to incorporate the effect of nonadiabatic coupling into the wave packet dynamics. This provides an interface between a general adiabatic frozen Gaussian wave packet propagation method and the trajectory surface hopping technique. The basic idea suggested in [A. D. Kondorskiy and H. Nakamura, J. Chem. Phys. 120, 8937 (2004)] is revisited and complemented in the present work by the elaboration of efficient numerical algorithms. We combine our approach with the adiabatic Herman-Kluk frozen Gaussian approximation. The efficiency and accuracy of the resulting method is demonstrated by applying it to popular benchmark model systems including three Tully's models and 24D model of pyrazine. It is shown that photoabsorption spectrum is successfully reproduced by using a few hundreds of trajectories. We employ the compact finite difference Hessian update scheme to consider feasibility of the ab initio "on-the-fly" simulations. It is found that this technique allows us to obtain the reliable final results using several Hessian matrix calculations per trajectory.

  4. Wave packet dynamics in doubly excited states of He

    NASA Astrophysics Data System (ADS)

    Feist, Johannes; Nagele, Stefan; Persson, Emil; Burgdörfer, Joachim; Schneider, Barry

    2007-06-01

    We have developed a method for the ab initio simulation of the interaction of ultrashort laser pulses with helium atoms. We expand the two-electron Schr"odinger equation in coupled spherical harmonics and perform direct time integration utilizing either the Arnoldi-Lanczos or the Leapfrog method. The spatial discretization is performed in an FEDVR basis [1]. This allows for a numerically accurate description while possessing desirable computational features, e.g. a block-diagonal form of the kinetic energy matrix. We will present results on electron-electron correlation and wave packet dynamics in He. By using a suitable combination of attosecond XUV/EUV pulses, we prepare a wave packet in the doubly excited states of helium. The motion of this wave packet can be observed by using a probe pulse to induce ionization. We aim for a detailed understanding of the process by a careful study of the ionized electrons, e.g. by investigating doubly differential momentum spectra. [enumi] *B. I. Schneider and L. A. Collins. J. Non-Cryst. Solids 351, 1551.

  5. Electronically nonadiabatic wave packet propagation using frozen Gaussian scattering

    SciTech Connect

    Kondorskiy, Alexey D.; Nanbu, Shinkoh

    2015-09-21

    We present an approach, which allows to employ the adiabatic wave packet propagation technique and semiclassical theory to treat the nonadiabatic processes by using trajectory hopping. The approach developed generates a bunch of hopping trajectories and gives all additional information to incorporate the effect of nonadiabatic coupling into the wave packet dynamics. This provides an interface between a general adiabatic frozen Gaussian wave packet propagation method and the trajectory surface hopping technique. The basic idea suggested in [A. D. Kondorskiy and H. Nakamura, J. Chem. Phys. 120, 8937 (2004)] is revisited and complemented in the present work by the elaboration of efficient numerical algorithms. We combine our approach with the adiabatic Herman-Kluk frozen Gaussian approximation. The efficiency and accuracy of the resulting method is demonstrated by applying it to popular benchmark model systems including three Tully’s models and 24D model of pyrazine. It is shown that photoabsorption spectrum is successfully reproduced by using a few hundreds of trajectories. We employ the compact finite difference Hessian update scheme to consider feasibility of the ab initio “on-the-fly” simulations. It is found that this technique allows us to obtain the reliable final results using several Hessian matrix calculations per trajectory.

  6. Generalized Gaussian wave packet dynamics: Integrable and chaotic systems.

    PubMed

    Pal, Harinder; Vyas, Manan; Tomsovic, Steven

    2016-01-01

    The ultimate semiclassical wave packet propagation technique is a complex, time-dependent Wentzel-Kramers-Brillouin method known as generalized Gaussian wave packet dynamics (GGWPD). It requires overcoming many technical difficulties in order to be carried out fully in practice. In its place roughly twenty years ago, linearized wave packet dynamics was generalized to methods that include sets of off-center, real trajectories for both classically integrable and chaotic dynamical systems that completely capture the dynamical transport. The connections between those methods and GGWPD are developed in a way that enables a far more practical implementation of GGWPD. The generally complex saddle-point trajectories at its foundation are found using a multidimensional Newton-Raphson root search method that begins with the set of off-center, real trajectories. This is possible because there is a one-to-one correspondence. The neighboring trajectories associated with each off-center, real trajectory form a path that crosses a unique saddle; there are exceptions that are straightforward to identify. The method is applied to the kicked rotor to demonstrate the accuracy improvement as a function of ℏ that comes with using the saddle-point trajectories. PMID:26871079

  7. Creating Rydberg electron wave packets using terahertz pulses

    NASA Astrophysics Data System (ADS)

    Bromage, Jake

    1999-10-01

    In this thesis I present experiments in which we excited classical-limit states of an atom using terahertz pulses. In a classical-limit state, an atom's outer electron is confined to a wave packet that orbits the core along a classical trajectory. Researchers have excited states with classical traits, but wave packets localized in all three dimensions have proved elusive. Theoretical studies have shown such states can be created using terahertz pulses. Using these techniques, we created a linear-orbit wave packet (LOWP), that is three-dimensionally localized and orbits along a line on one side of the atom's core. Terahertz pulses are sub-picosecond bursts of far- infrared radiation. Unlike ultrashort optical pulses, the electric field of terahertz pulses barely completes a single cycle. Our simulations of the atom-pulse interaction show that this electric field profile is critical in determining the quality of the wave packet. To characterize our terahertz pulses, we invented dithered-edge sampling which time- resolves the electric field using a photoconductive receiver and a triggered attenuator. We also studied how pulses are distorted after propagating through metallic structures, and used our findings to design our atomic experiments. We excited wave packets in atomic sodium using a two-step process. First, we used tunable, nanosecond dye lasers to excite an extreme Stark state. Next, we used a terahertz pump pulse to coherently redistribute population among extreme Stark states in neighboring manifolds. Interference between the final states produces a localized, dynamic LOWP. To analyze the LOWP, we ionized it with a stronger terahertz probe pulse, varying the pump-probe delay to map out its motion. We observed two strong LOWP signatures. Changing the static electric field produced small changes (2%) in the orbital period that agreed with our theoretical predictions. Secondly, because the LOWP scatters off the core, the pump-probe signal depended on the

  8. Engineering biphoton wave packets with an electromagnetically induced grating

    SciTech Connect

    Wen Jianming; Xiao Min; Zhai Yanhua; Du Shengwang

    2010-10-15

    We propose to shape biphoton wave packets with an electromagnetically induced grating in a four-level double-{Lambda} cold atomic system. We show that the induced hybrid grating plays an essential role in directing the new fields into different angular positions, especially for the zeroth-order diffraction. A number of interesting features appears in the shaped two-photon wave forms. For example, broadening or narrowing the spectrum would be possible in the proposed scheme even without the use of a cavity.

  9. Wave-packet evolution in non-Hermitian quantum systems

    SciTech Connect

    Graefe, Eva-Maria; Schubert, Roman

    2011-06-15

    The quantum evolution of the Wigner function for Gaussian wave packets generated by a non-Hermitian Hamiltonian is investigated. In the semiclassical limit ({h_bar}/2{pi}){yields}0 this yields the non-Hermitian analog of the Ehrenfest theorem for the dynamics of observable expectation values. The lack of Hermiticity reveals the importance of the complex structure on the classical phase space: The resulting equations of motion are coupled to an equation of motion for the phase-space metric - a phenomenon having no analog in Hermitian theories.

  10. Selection of ionization paths of K2 on superfluid helium droplets by wave packet interference

    NASA Astrophysics Data System (ADS)

    Hild, Marek Bastian; Dufour, Adrien; Achazi, Georg; Patas, Alexander; Scheier, Paul; Lindinger, Albrecht

    2016-08-01

    We report on the control of wave packet dynamics for the ionization of K2 attached to the surface of superfluid helium droplets. The superfluid helium matrix acts as a heat sink and reduces the coherence time of molecular processes by dissipation. We use tailor-shaped pulses in order to activate or inhibit different ionization paths by constructive or destructive wave packet interference. A drastic change of the wave packet dynamics is observed by shifting the phase between the exciting sub pulses.

  11. Encoding and Decoding Information in High-n Circular Wave Packets

    SciTech Connect

    Yoshida, S.; Reinhold, Carlos O; Burgdorfer, J.; Wyker, B.; Dunning, F. B.

    2010-01-01

    We demonstrate theoretically and experimentally the extraction of detailed information on the density matrix of very-high-n(> 300) near-circular Rydberg wave packets through Fourier analysis of the quantum beat and quantum revival signal. The remarkably long coherence times associated with circular wave packets facilitate the preservation and read-out of information encoded in this matrix. We illustrate the power of the method by determining the angular localization of the components of a wave packet.

  12. Time behavior of a Gaussian wave packet accompanying the generalized coherent state for the inverted oscillator

    NASA Astrophysics Data System (ADS)

    Maamache, Mustapha; Bouguerra, Yacine; Choi, Jeong Ryeol

    2016-06-01

    A Gaussian wave packet of the inverted oscillator is investigated using the invariant operator method together with the unitary transformation method. A simple wave packet directly derived from the eigenstates of the invariant operator of the system corresponds to a plane wave that is fully delocalized. However, we can construct a weighted wave packet in terms of such plane waves, which corresponds to a Gaussian wave. This wave packet is associated with the generalized coherent state, which can be crucially utilized for investigating the classical limit of quantum wave mechanics. Various quantum properties of the system, such as fluctuations of the canonical variables, the uncertainty product, and the motion of the wave packet or quantum particle, are analyzed by means of this wave packet. We have confirmed that the time behavior of such a wave packet is very similar to the counterpart classical state. The wave packet runs away from the origin in the positive or negative direction in the 1D coordinate depending on the condition of the initial state. We have confirmed that this wave packet not only moves acceleratively but also spreads out during its propagation.

  13. Wave-packet dynamics on Chern-band lattices in a trap

    NASA Astrophysics Data System (ADS)

    Roy, Sthitadhi; Grushin, Adolfo G.; Moessner, Roderich; Haque, Masudul

    2015-12-01

    The experimental realization of lattices with Chern bands in ultracold-atom and photonic systems has motivated the study of time-dependent phenomena, such as spatial propagation, in lattices with nontrivial topology. We study the dynamics of Gaussian wave packets on the Haldane honeycomb Chern-band lattice model, in the presence of a harmonic trap. We focus on the transverse response to a force, which is due partly to the Berry curvature and partly to the transverse component of the energy band curvature. We evaluate the accuracy of a semiclassical description, which treats the wave packet as a point particle in both real and momentum space, in reproducing the motion of a realistic wave packet with finite extent. We find that, in order to accurately capture the wave-packet dynamics, the extent of the wave packet in momentum space needs to be taken into account: The dynamics is sensitive to the interplay of band dispersion and Berry curvature over the finite region of momentum (reciprocal) space where the wave packet has support. Moreover, if the wave packet is prepared with a finite initial momentum, the semiclassical analysis reproduces its motion as long as it has a large overlap with the eigenstates of a single band. The semiclassical description generally improves with increasing real-space size of the wave packet, as long as the external conditions (e.g., external force) remain uniform throughout the spatial extent of the wave packet.

  14. Field structure of collapsing wave packets in 3D strong Langmuir turbulence

    NASA Technical Reports Server (NTRS)

    Newman, D. L.; Robinson, P. A.; Goldman, M. V.

    1989-01-01

    A simple model is constructed for the electric fields in the collapsing wave packets found in 3D simulations of driven and damped isotropic strong Langmuir turbulence. This model, based on a spherical-harmonic decomposition of the electrostatic potential, accounts for the distribution of wave-packet shapes observed in the simulations, particularly the predominance of oblate wave packets. In contrast with predictions for undamped and undriven subsonic collapse of scalar fields, oblate vector-field wave packets do not flatten during collapse but, instead, remain approximately self-similar and rigid.

  15. Fokker-Planck electron diffusion caused by an obliquely propagating electromagnetic wave packet of narrow bandwidth

    NASA Technical Reports Server (NTRS)

    Hizanidis, Kyriakos

    1989-01-01

    The relativistic motion of electrons in an intense electromagnetic wave packet propagating obliquely to a uniform magnetic field is analytically studied on the basis of the Fokker-Planck-Kolmogorov (FPK) approach. The wavepacket consists of circularly polarized electron-cyclotron waves. The dynamical system in question is shown to be reducible to one with three degrees of freedom. Within the framework of the Hamiltonian analysis the nonlinear diffusion tensor is derived, and it is shown that this tensor can be separated into zeroth-, first-, and second-order parts with respect to the relative bandwidth. The zeroth-order part describes diffusive acceleration along lines of constant unperturbed Hamiltonian. The second-order part, which corresponds to the longest time scale, describes diffusion across those lines. A possible transport theory is outlined on the basis of this separation of the time scales.

  16. Transport of time-varying plasma currents by whistler wave packets

    NASA Technical Reports Server (NTRS)

    Stenzel, R. L.; Urrutia, J. M.; Rousculp, C.

    1992-01-01

    The relationship between pulsed currents and electromagnetic waves is examined in a regime characterized by electron MHD. Pulsed currents are generated by (1) collection/emission of charged particles by/from biased electrodes and (2) induction of currents by time-varying and moving magnetic fields. Pulsed currents are observed to propagate at the speed of whistler wave packets. Their field structure forms ropelike configurations which are electromagnetically force-free. Moving sources induce 'eddy' currents which excite waves and form Cerenkov-like whistler 'wings'. The radiation patterns of moving magnetic antennas and electrodynamic tethers are investigated. Nonlinear effects of large-amplitude, antenna-launched whistler pulses are observed. These involve a new modulational instability in which a channel of high conductivity which permits the wave/currents to penetrate deeply into a collisional plasma is formed.

  17. Wave packet simulations of phonon boundary scattering at graphene edges

    NASA Astrophysics Data System (ADS)

    Wei, Zhiyong; Chen, Yunfei; Dames, Chris

    2012-07-01

    Wave packet dynamics is used to investigate the scattering of longitudinal (LA), transverse (TA), and bending-mode (ZA) phonons at the zigzag and armchair edges of suspended graphene. The interatomic forces are calculated using a linearized Tersoff potential. The strength of a boundary scattering event at impeding energy flow is described by a forward scattering coefficient, similar in spirit to a specularity parameter. For armchair boundaries, this scattering coefficient is found to depend strongly on the magnitude, direction, and polarization of the incident wavevector, while for zigzag boundaries, the forward scattering coefficient is found to always be unity regardless of wavevector and polarization. Wave packet splitting is observed for ZA phonons incident on armchair boundaries, while both splitting and mode conversion are observed for LA and TA phonons incident on both zigzag and armchair boundaries. These simulation results show that armchair boundaries impede the forward propagation of acoustic phonon energy much more strongly than zigzag boundaries do, suggesting that graphene nanoribbons will have substantially lower thermal conductivity in armchair rather than zigzag orientation.

  18. Creation of multihole molecular wave packets via strong-field ionization

    SciTech Connect

    Geissler, Dominik; Weinacht, Thomas; Rozgonyi, Tamas; Gonzalez-Vazquez, Jesus; Gonzalez, Leticia; Nichols, Sarah

    2010-07-15

    We demonstrate the creation of vibrational wave packets on multiple electronic states of a molecule via strong-field ionization. Furthermore, we show that the relative contribution of the different electronic states depends on the shape of the laser pulse which launches the wave packets.

  19. On the Behavior of Three-dimensional Wave Packets in Viscously Spreading Mixing Layers

    NASA Technical Reports Server (NTRS)

    Balsa, Thomas F.

    1994-01-01

    We consider analytically the evolution of a three-dimensional wave packet generated by an impulsive source in a mixing layer. The base flow is assumed to be spreading due to viscous diffusion. The analysis is restricted to small disturbances (linearized theory). A suitable high-frequency ansatz is used to describe the packet; the key elements of this description are a complex phase and a wave action density. It is found that the product of this density and an infinitesimal material volume convecting at the local group velocity is not conserved: there is a continuous interaction between the base flow and the wave action. This interaction is determined by suitable mode-weighted averages of the second and fourth derivatives of the base-flow velocity profile. Although there is some tendency for the dominant wave number in the packet to shift from the most unstable value toward the neutral value, this shift is quite moderate. In practice, wave packets do not become locally neutral in a diverging base flow (as do instability modes), therefore, they are expected to grow more suddenly than pure instability modes and do not develop critical layers. The group velocity is complex; the full significance of this is realized by analytically continuing the equations for the phase and wave action into a complex domain. The implications of this analytic continuation are discussed vis-a-vis the secondary instabilities of the packet: very small scale perturbations on the phase can grow very rapidly initially, but saturate later because most of the energy in these perturbations is convected away by the group velocity. This remark, as well as the one regarding critical layers, has consequences for the nonlinear theories.

  20. On the behavior of three-dimensional wave packets in viscously spreading mixing layers

    NASA Astrophysics Data System (ADS)

    Balsa, Thomas F.

    1994-11-01

    We consider analytically the evolution of a three-dimensional wave packet generated by an impulsive source in a mixing layer. The base flow is assumed to be spreading due to viscous diffusion. The analysis is restricted to small disturbances (linearized theory). A suitable high-frequency ansatz is used to describe the packet; the key elements of this description are a complex phase and a wave action density. It is found that the product of this density and an infinitesimal material volume convecting at the local group velocity is not conserved: there is a continuous interaction between the base flow and the wave action. This interaction is determined by suitable mode-weighted averages of the second and fourth derivatives of the base-flow velocity profile. Although there is some tendency for the dominant wave number in the packet to shift from the most unstable value toward the neutral value, this shift is quite moderate. In practice, wave packets do not become locally neutral in a diverging base flow (as do instability modes), therefore, they are expected to grow more suddenly than pure instability modes and do not develop critical layers. The group velocity is complex; the full significance of this is realized by analytically continuing the equations for the phase and wave action into a complex domain. The implications of this analytic continuation are discussed vis-a-vis the secondary instabilities of the packet: very small scale perturbations on the phase can grow very rapidly initially, but saturate later because most of the energy in these perturbations is convected away by the group velocity. This remark, as well as the one regarding critical layers, has consequences for the nonlinear theories.

  1. Magnetic helicity conservation and inverse energy cascade in electron magnetohydrodynamic wave packets.

    PubMed

    Cho, Jungyeon

    2011-05-13

    Electron magnetohydrodynamics (EMHD) provides a fluidlike description of small-scale magnetized plasmas. An EMHD wave propagates along magnetic field lines. The direction of propagation can be either parallel or antiparallel to the magnetic field lines. We numerically study propagation of three-dimensional (3D) EMHD wave packets moving in one direction. We obtain two major results. (1) Unlike its magnetohydrodynamic (MHD) counterpart, an EMHD wave packet is dispersive. Because of this, EMHD wave packets traveling in one direction create opposite-traveling wave packets via self-interaction and cascade energy to smaller scales. (2) EMHD wave packets traveling in one direction clearly exhibit inverse energy cascade. We find that the latter is due to conservation of magnetic helicity. We compare inverse energy cascade in 3D EMHD turbulence and two-dimensional (2D) hydrodynamic turbulence. PMID:21668138

  2. Magnetic Helicity Conservation and Inverse Energy Cascade in Electron Magnetohydrodynamic Wave Packets

    SciTech Connect

    Cho, Jungyeon

    2011-05-13

    Electron magnetohydrodynamics (EMHD) provides a fluidlike description of small-scale magnetized plasmas. An EMHD wave propagates along magnetic field lines. The direction of propagation can be either parallel or antiparallel to the magnetic field lines. We numerically study propagation of three-dimensional (3D) EMHD wave packets moving in one direction. We obtain two major results. (1) Unlike its magnetohydrodynamic (MHD) counterpart, an EMHD wave packet is dispersive. Because of this, EMHD wave packets traveling in one direction create opposite-traveling wave packets via self-interaction and cascade energy to smaller scales. (2) EMHD wave packets traveling in one direction clearly exhibit inverse energy cascade. We find that the latter is due to conservation of magnetic helicity. We compare inverse energy cascade in 3D EMHD turbulence and two-dimensional (2D) hydrodynamic turbulence.

  3. Flavor entanglement in neutrino oscillations in the wave packet description

    NASA Astrophysics Data System (ADS)

    Blasone, Massimo; Dell'Anno, Fabio; De Siena, Silvio; Illuminati, Fabrizio

    2015-10-01

    The wave packet approach to neutrino oscillations provides an enlightening description of quantum decoherence induced, during propagation, by localization effects. Within this approach, we show that a deeper insight into the dynamical aspects of particle mixing can be obtained if one investigates the behavior of quantum correlations associated to flavor oscillations. By identifying the neutrino three-flavor modes with (suitably defined) three-qubit modes, the exploitation of tools of quantum information theory for mixed states allows a detailed analysis of the dynamical behavior of flavor entanglement during free propagation. This provides further elements leading to a more complete understanding of the phenomenon of neutrino oscillations, and a basis for possible applicative implementations. The analysis is carried out by studying the distribution of the flavor entanglement; to this aim, we perform combined investigations of the behaviors of the two-flavor concurrence and of the logarithmic negativities associated with specific bipartitions of the three flavors.

  4. Diffraction using laser-driven broadband electron wave packets

    NASA Astrophysics Data System (ADS)

    Xu, Junliang; Blaga, Cosmin I.; Zhang, Kaikai; Lai, Yu Hang; Lin, C. D.; Miller, Terry A.; Agostini, Pierre; Dimauro, Louis F.

    2014-08-01

    Directly monitoring atomic motion during a molecular transformation with atomic-scale spatio-temporal resolution is a frontier of ultrafast optical science and physical chemistry. Here we provide the foundation for a new imaging method, fixed-angle broadband laser-induced electron scattering, based on structural retrieval by direct one-dimensional Fourier transform of a photoelectron energy distribution observed along the polarization direction of an intense ultrafast light pulse. The approach exploits the scattering of a broadband wave packet created by strong-field tunnel ionization to self-interrogate the molecular structure with picometre spatial resolution and bond specificity. With its inherent femtosecond resolution, combining our technique with molecular alignment can, in principle, provide the basis for time-resolved tomography for multi-dimensional transient structural determination.

  5. Diffraction using laser-driven broadband electron wave packets

    NASA Astrophysics Data System (ADS)

    Xu, Junliang; Blaga, Cosmin I.; Zhang, Kaikai; Lai, Yu Hang; Lin, C. D.; Miller, Terry A.; Agostini, Pierre; Dimauro, Louis F.

    2015-05-01

    Directly monitoring atomic motion during a molecular transformation with atomic-scale spatio-temporal resolution is a frontier of ultrafast optical science and physical chemistry. Here we provide the foundation for a new imaging method, fixed-angle broadband laser-induced electron scattering, based on structural retrieval by direct one-dimensional Fourier transform of a photoelectron energy distribution observed along the polarization direction of an intense ultrafast light pulse. The approach exploits the scattering of a broadband wave packet created by strong-field tunnel ionization to self-interrogate the molecular structure with picometer spatial resolution and bond specificity. With its inherent femtosecond resolution, combining our technique with molecular alignment can, in principle, provide the basis for time-resolved tomography for multi-dimensional transient structural determination.

  6. Quantum oscillations and wave packet revival in conical graphene structure

    NASA Astrophysics Data System (ADS)

    Sinha, Debabrata; Berche, Bertrand

    2016-03-01

    We present analytical expressions for the eigenstates and eigenvalues of electrons confined in a graphene monolayer in which the crystal symmetry is locally modified by replacing a hexagon by a pentagon, square or heptagon. The calculations are performed in the continuum limit approximation in the vicinity of the Dirac points, solving Dirac equation by freezing out the carrier radial motion. We include the effect of an external magnetic field and show the appearance of Aharonov-Bohm oscillations and find out the conditions of gapped and gapless states in the spectrum. We show that the gauge field due to a disclination lifts the orbital degeneracy originating from the existence of two valleys. The broken valley degeneracy has a clear signature on quantum oscillations and wave packet dynamics.

  7. Hydrodynamic view of wave-packet interference: quantum caves.

    PubMed

    Chou, Chia-Chun; Sanz, Angel S; Miret-Artés, Salvador; Wyatt, Robert E

    2009-06-26

    Wave-packet interference is investigated within the complex quantum Hamilton-Jacobi formalism using a hydrodynamic description. Quantum interference leads to the formation of the topological structure of quantum caves in space-time Argand plots. These caves consist of the vortical and stagnation tubes originating from the isosurfaces of the amplitude of the wave function and its first derivative. Complex quantum trajectories display counterclockwise helical wrapping around the stagnation tubes and hyperbolic deflection near the vortical tubes. The string of alternating stagnation and vortical tubes is sufficient to generate divergent trajectories. Moreover, the average wrapping time for trajectories and the rotational rate of the nodal line in the complex plane can be used to define the lifetime for interference features. PMID:19659057

  8. Simulation of wave packet tunneling of interacting identical particles

    NASA Astrophysics Data System (ADS)

    Lozovik, Yu. E.; Filinov, A. V.; Arkhipov, A. S.

    2003-02-01

    We demonstrate a different method of simulation of nonstationary quantum processes, considering the tunneling of two interacting identical particles, represented by wave packets. The used method of quantum molecular dynamics (WMD) is based on the Wigner representation of quantum mechanics. In the context of this method ensembles of classical trajectories are used to solve quantum Wigner-Liouville equation. These classical trajectories obey Hamiltonian-like equations, where the effective potential consists of the usual classical term and the quantum term, which depends on the Wigner function and its derivatives. The quantum term is calculated using local distribution of trajectories in phase space, therefore, classical trajectories are not independent, contrary to classical molecular dynamics. The developed WMD method takes into account the influence of exchange and interaction between particles. The role of direct and exchange interactions in tunneling is analyzed. The tunneling times for interacting particles are calculated.

  9. Decoherence of wave packets in an anharmonic oscillator

    SciTech Connect

    Foeldi, Peter; Benedict, Mihaly G.; Czirjak, Attila; Molnar, Balazs

    2003-03-01

    The time evolution of wave packets in the Morse potential is investigated under the influence of the environment consisting of harmonic oscillators. These oscillators represent photon or phonon modes and are assumed to be in thermal equilibrium. Our model explicitly incorporates the fact that in the case of a nonequidistant spectrum the rates of the environment induced transitions are different for each transition. The nonunitary time evolution is visualized by the aid of the corresponding Wigner function. The time scale of decoherence is much shorter than that of dissipation, and gives rise to states that are mixtures of localized states along the phase-space orbit of the corresponding classical particle. This behavior is to a large extent independent of the coupling strength, the temperature of the environment, and also the initial state.

  10. Nonlinear Kalman filters for calibration in radio interferometry

    NASA Astrophysics Data System (ADS)

    Tasse, C.

    2014-06-01

    The data produced by the new generation of interferometers are affected by a wide variety of partially unknown complex effects such as pointing errors, phased array beams, ionosphere, troposphere, Faraday rotation, or clock drifts. Most algorithms addressing direction-dependent calibration solve for the effective Jones matrices, and cannot constrain the underlying physical quantities of the radio interferometry measurement equation (RIME). A related difficulty is that they lack robustness in the presence of low signal-to-noise ratios, and when solving for moderate to large numbers of parameters they can be subject to ill-conditioning. These effects can have dramatic consequences in the image plane such as source or even thermal noise suppression. The advantage of solvers directly estimating the physical terms appearing in the RIME is that they can potentially reduce the number of free parameters by orders of magnitudes while dramatically increasing the size of usable data, thereby improving conditioning. We present here a new calibration scheme based on a nonlinear version of the Kalman filter that aims at estimating the physical terms appearing in the RIME. We enrich the filter's structure with a tunable data representation model, together with an augmented measurement model for regularization. Using simulations we show that it can properly estimate the physical effects appearing in the RIME. We found that this approach is particularly useful in the most extreme cases such as when ionospheric and clock effects are simultaneously present. Combined with the ability to provide prior knowledge on the expected structure of the physical instrumental effects (expected physical state and dynamics), we obtain a fairly computationally cheap algorithm that we believe to be robust, especially in low signal-to-noise regimes. Potentially, the use of filters and other similar methods can represent an improvement for calibration in radio interferometry, under the condition that

  11. Theory and experiment of coherent wave packet dynamics in rare earth solids: Absorption spectrum vs femtosecond fringe-resolved interferogram

    NASA Astrophysics Data System (ADS)

    Luo, Q.; Dai, D. C.; Wang, G. Q.; Ninulescu, V.; Yu, X. Y.; Luo, L.; Zhou, J. Y.; Yan, YiJing

    2001-01-01

    Coherent dynamic property of neodymium yttrium aluminum garnet (Nd:YAG) crystal at 77 K is studied via the conventional absorption, the femtosecond fringe-resolved wave packet interferometry, and the related difference-phase spectrum. The recorded interferogram exhibits beatings in subpicosecond time scale arising from the interferences among various weakly split 4f-electronic states and the coupled vibronic optical phonon sidebands. The electron-phonon coupling in Nd:YAG can be well described by multiple Brownian oscillators model involving in each individual electronic transition. The parameters for characterizing material coherence and relaxation are determined via the theoretical modelings of both the frequency and the time-domain experimental signals.

  12. Eliminating the dipole phase in attosecond pulse characterization using Rydberg wave packets

    NASA Astrophysics Data System (ADS)

    Pabst, Stefan; Dahlström, Jan Marcus

    2016-07-01

    We propose a technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wave packet. The influence of the dipole phase, which is the main obstacle for state-of-the-art pulse characterization schemes, can be eliminated by angle integration of the photoelectron spectrum. We show that in particular, atomic Rydberg wave packets are ideal and that wave packets involving multiple electronic states provide redundant information that can be used to cross-check the consistency of the phase reconstruction.

  13. Theory of probing attosecond electron wave packets via two-path interference of angle-resolved photoelectrons

    SciTech Connect

    Choi, N. N.; Jiang, T. F.; Morishita, T.; Lee, M.-H.; Lin, C. D.

    2010-07-15

    We study theoretically the electron wave packet generated by an attosecond pulse train (APT) which is probed with a time-delayed infrared (IR) laser pulse. The APT creates an excited state and a continuum electron wave packet. By ionizing the excited state with an IR, a delayed new continuum electron wave packet is created. The interference of the wave packets from the two paths, as reflected in angle-resolved photoelectron spectra, is analyzed analytically. Using the analytical expressions, we examine the possibility of retrieving information on the electron wave packet generated by the APT.

  14. The evolution of a breaking mesospheric bore wave packet

    NASA Astrophysics Data System (ADS)

    Stockwell, R. G.; Taylor, M. J.; Nielsen, K.; Jarvis, M. J.

    2011-10-01

    All-sky CCD observations of mesospheric gravity waves have been made from Halley Station Antarctica (75.5°S, 26.7°W) as part of a collaborative research program between British Antarctic Survey, U.K. and Utah State University, USA. A mesospheric bore event was observed in the nightglow emissions over a period of several hours on the 27th of May, 2001. Two dimensional S-Transform (ST) analysis is applied to the airglow images of this bore event. This local spectral technique allows one to calculate the wave parameters as a function of time and space. It is observed that the horizontal phase speed and wavelength decrease over time as the amplitude attenuates. Simultaneously with this wave event the background wind experiences a large acceleration in the direction of the wave propagation. Mesospheric bore theory calculations are used to estimate the bore duct depth and it is shown that as the wave packet evolves, the bore duct collapses (decreasing in its vertical extent). As the bore duct shrinks, the wave's group velocity decelerates, the amplitude attenuates, and the wave dissipates.

  15. Riemann {zeta} function from wave-packet dynamics

    SciTech Connect

    Mack, R.; Schleich, W. P.; Dahl, J. P.; Moya-Cessa, H.; Strunz, W. T.; Walser, R.

    2010-09-15

    We show that the time evolution of a thermal phase state of an anharmonic oscillator with logarithmic energy spectrum is intimately connected to the generalized Riemann {zeta} function {zeta}(s,a). Indeed, the autocorrelation function at a time t is determined by {zeta}({sigma}+i{tau},a), where {sigma} is governed by the temperature of the thermal phase state and {tau} is proportional to t. We use the JWKB method to solve the inverse spectral problem for a general logarithmic energy spectrum; that is, we determine a family of potentials giving rise to such a spectrum. For large distances, all potentials display a universal behavior; they take the shape of a logarithm. However, their form close to the origin depends on the value of the Hurwitz parameter a in {zeta}(s,a). In particular, we establish a connection between the value of the potential energy at its minimum, the Hurwitz parameter and the Maslov index of JWKB. We compare and contrast exact and approximate eigenvalues of purely logarithmic potentials. Moreover, we use a numerical method to find a potential which leads to exact logarithmic eigenvalues. We discuss possible realizations of Riemann {zeta} wave-packet dynamics using cold atoms in appropriately tailored light fields.

  16. Alfvénic wave packets collision in a kinetic plasma

    NASA Astrophysics Data System (ADS)

    Pezzi, Oreste; Parashar, Tulasi N.; Servidio, Sergio; Valentini, Francesco; Malara, Francesco; Matthaeus, William H.; Veltri, Pierluigi

    2016-04-01

    The problem of two colliding and counter-propagating Alfvénic wave packets has been investigated in detail since the late Seventies. In particular Moffatt [1] and Parker [2] showed that, in the framework of the incompressible magnetohydrodynamics (MHD), nonlinear interactions can develop only during the overlapping of the two packets. Here we describe a similar problem in the framework of the kinetic physics. The collision of two quasi-Alfvénic packets has been analyzed by means of MHD, Hall-MHD and kinetic simulations performed with two different hybrid codes: a PIC code [3] and a Vlasov-Maxwell code [4]. Due to the huge computational cost, only a 2D-3V phase space is allowed (two dimensions in the physical space, three dimensions in the velocity space). Preliminary results suggest that, as well as in the MHD case, the most relevant nonlinear effects occur during the overlapping of the two packets. For both the PIC and Vlasov cases, strong temperature anisotropies are present during the evolution of the wave packets. Moreover, due to the absence of numerical noise, Vlasov simulations show that the collision of the counter-propagating solitary waves produces a significant beam in the velocity distribution functions [5], which, instead, cannot be appreciated in PIC simulations. We remark that, beyond the interest of studying a well-known MHD problem in the realm of the kinetic physics, our results allows also to compare different numerical codes. [1] H.K. Moffatt, Field generation in electrically conducting fluids (Cambridge University Press, 1978). [2] E.N. Parker, Cosmical magnetic fields: their origin and their activity (Oxford University Press, 1979). [3] T.N. Parashar, M.A. Shay, P.A. Cassak and W.H. Matthaeus, Physics of Plasmas 16, 032310 (2009). [4] F. Valentini, P. Trávníček, F. Califano, P. Hellinger & A. Mangeney, Journal of Computational Physics 225, 753-770 (2007). [5] J. He, C. Tu, E. Marsch, C.H. Chen, L. Wang, Z. Pei, L. Zhang, C.S. Salem and S

  17. Femtosecond wave-packet dynamics in cesium dimers studied through controlled stimulated emission

    SciTech Connect

    Yuan Luqi; Wang Xi; Patnaik, Anil K.; Sokolov, Alexei V.; Ariunbold, Gombojav O.; Murawski, Robert K.; Pestov, Dmitry; Sautenkov, Vladimir A.; Rostovtsev, Yuri V.; Scully, Marlan O.

    2010-05-15

    We study the dynamics of wave packets in cesium dimers using a femtosecond-controlled pump-probe technique. We implement configurations with one pulse (pump) or two pulses (pump and control) to produce vibrational wave packets on the electronic excited state. The transmission of an additional, variable-delay probe pulse is measured to monitor the time evolution of the wave packets. In the case of the pump-control-probe configuration, a superposition of two independent wave packets is observed. In order to elucidate the observed experimental data, we develop a theory based on the Liouville equation for the density matrix associated with the Franck-Condon factors. Both the numerical and analytical calculations are in good agreement with our experimental results.

  18. Temporal and spatial manipulation of the recolliding wave packet in strong-field photoelectron holography

    NASA Astrophysics Data System (ADS)

    He, Mingrui; Li, Yang; Zhou, Yueming; Li, Min; Lu, Peixiang

    2016-03-01

    We theoretically demonstrate temporal and spatial manipulation of electron wave packets involved in strong-field photoelectron holography (SFPH) with the orthogonally polarized two-color laser fields. By varying the relative phase of the two-color fields, the recollision time of the returning wave packet can be accurately controlled, which allows us to switch off and on the holographic interference. Moreover, the recollision angles of the returning electron wave packet can be arbitrarily controlled via changing the relative intensity of the two-color fields, and thus the structure information of the target is encoded in the hologram by the recollision electron wave packet from different angles. This makes the SFPH a powerful technique of imaging the molecular structure as well as ultrafast dynamics on an attosecond time scale.

  19. Quantum-Phase Resolved Mapping of Ground-State Vibrational D{sub 2} Wave Packets via Selective Depletion in Intense Laser Pulses

    SciTech Connect

    Ergler, Th.; Rudenko, A.; Schroeter, C. D.; Moshammer, R.; Ullrich, J.; Feuerstein, B.; Zrost, K.

    2006-09-08

    Applying 7 fs pump-probe pulses (780 nm, 4x10{sup 14} W/cm{sup 2}) we observe electronic ground-state vibrational wave packets in neutral D{sub 2} with a period of T=11.101(70) fs by following the internuclear separation (R-)dependent ionization with a sensitivity of {delta}{<=}0.02 A . The absolute phase of the wave packet's motion provides evidence for R-dependent depletion of the ground state by nonlinear ionization, to be the dominant preparation mechanism. A phase shift of about {pi} found between pure ionization (D{sub 2}{sup +}) and dissociation (D{sup +}+D) channels opens a pathway of quantum control.

  20. Spontaneous emission of a photon: Wave-packet structures and atom-photon entanglement

    SciTech Connect

    Fedorov, M.V.; Efremov, M.A.; Kazakov, A.E.; Chan, K.W.; Eberly, J.H.; Law, C.K.

    2005-09-15

    Spontaneous emission of a photon by an atom is described theoretically in three dimensions with the initial wave function of a finite-mass atom taken in the form of a finite-size wave packet. Recoil and wave-packet spreading are taken into account. The total atom-photon wave function is found in the momentum and coordinate representations as the solution of an initial-value problem. The atom-photon entanglement arising in such a process is shown to be closely related to the structure of atom and photon wave packets which can be measured in the coincidence and single-particle schemes of measurements. Two predicted effects, arising under the conditions of high entanglement, are anomalous narrowing of the coincidence wave packets and, under different conditions, anomalous broadening of the single-particle wave packets. Fundamental symmetry relations between the photon and atom single-particle and coincidence wave-packet widths are established. The relationship with the famous scenario of Einstein-Podolsky-Rosen is discussed.

  1. Observation of Wave Packet Distortion during a Negative-Group-Velocity Transmission

    PubMed Central

    Ye, Dexin; Salamin, Yannick; Huangfu, Jiangtao; Qiao, Shan; Zheng, Guoan; Ran, Lixin

    2015-01-01

    In Physics, causality is a fundamental postulation arising from the second law of thermodynamics. It states that, the cause of an event precedes its effect. In the context of Electromagnetics, the relativistic causality limits the upper bound of the velocity of information, which is carried by electromagnetic wave packets, to the speed of light in free space (c). In anomalously dispersive media (ADM), it has been shown that, wave packets appear to propagate with a superluminal or even negative group velocity. However, Sommerfeld and Brillouin pointed out that the “front” of such wave packets, known as the initial point of the Sommerfeld precursor, always travels at c. In this work, we investigate the negative-group-velocity transmission of half-sine wave packets. We experimentally observe the wave front and the distortion of modulated wave packets propagating with a negative group velocity in a passive artificial ADM in microwave regime. Different from previous literature on the propagation of superluminal Gaussian packets, strongly distorted sinusoidal packets with non-superluminal wave fronts were observed. This result agrees with Brillouin's assertion, i.e., the severe distortion of seemingly superluminal wave packets makes the definition of group velocity physically meaningless in the anomalously dispersive region. PMID:25631746

  2. Observation of wave packet distortion during a negative-group-velocity transmission.

    PubMed

    Ye, Dexin; Salamin, Yannick; Huangfu, Jiangtao; Qiao, Shan; Zheng, Guoan; Ran, Lixin

    2015-01-01

    In Physics, causality is a fundamental postulation arising from the second law of thermodynamics. It states that, the cause of an event precedes its effect. In the context of Electromagnetics, the relativistic causality limits the upper bound of the velocity of information, which is carried by electromagnetic wave packets, to the speed of light in free space (c). In anomalously dispersive media (ADM), it has been shown that, wave packets appear to propagate with a superluminal or even negative group velocity. However, Sommerfeld and Brillouin pointed out that the "front" of such wave packets, known as the initial point of the Sommerfeld precursor, always travels at c. In this work, we investigate the negative-group-velocity transmission of half-sine wave packets. We experimentally observe the wave front and the distortion of modulated wave packets propagating with a negative group velocity in a passive artificial ADM in microwave regime. Different from previous literature on the propagation of superluminal Gaussian packets, strongly distorted sinusoidal packets with non-superluminal wave fronts were observed. This result agrees with Brillouin's assertion, i.e., the severe distortion of seemingly superluminal wave packets makes the definition of group velocity physically meaningless in the anomalously dispersive region. PMID:25631746

  3. Reduction of a wave packet in quantum Brownian motion

    NASA Astrophysics Data System (ADS)

    Unruh, W. G.; Zurek, W. H.

    1989-08-01

    The effect of the environment on a quantum system is studied on an exactly solvable model: a harmonic oscillator interacting with a one-dimensional massless scalar field. We show that in an open quantum system, dissipation can cause decorrelation on a time scale significantly shorter than the relaxation time which characterizes the approach of the system to thermodynamic equilibrium. In particular, we demonstrate that the density matrix decays rapidly toward a mixture of ``approximate eigenstates'' of the ``pointer observable,'' which commutes with the system-environment interaction Hamiltonian. This observable can be regarded as continuously, if inaccurately, monitored by the scalar field environment. Both because in a harmonic oscillator the state of the system rotates in the phase space and because the effective environment ``measurement'' is weak, the system, on the short ``collision'' time scale (1/Γ), maintains a coherence in this pointer observable on time scales of order [γ/Ωln(Γ/Ω)]1/2 and on longer time scales settles into a mixture of coherent states with a dispersion approximately consistent with the vacuum state. The master equation satisfied by the exact solution differs from the other master equations derived both for the high-temperature limit and for T=0. We discuss these differences and study the transition region between the high- and low-temperature regimes. We also consider the behavior of the system in the short-time ``transient'' regime. For T=0, we find that, in the long-time limit, the system behaves as if it were subject to ``1/f noise.'' The generality of our model is considered and its predictions are compared with previous treatments of related problems. Some of the possible applications of the results to experimentally realizable situations are outlined. The significance of the environment-induced reduction of the wave packet for cosmological models is also briefly considered.

  4. Correlation of femtosecond wave packets and fluorescence interference in a conjugated polymer: Towards the measurement of site homogeneous dephasing

    NASA Astrophysics Data System (ADS)

    Milota, F.; Sperling, J.; Szöcs, V.; Tortschanoff, A.; Kauffmann, H. F.

    2004-05-01

    Probing electronic femtosecond (fs) coherence among segmental sites that are congested by static and dynamic site disorder and subject to structural relaxation is a big, experimental challenge in the study of photophysics of poly(p-phenylenevinylene). In this work, fs-wave-packet fluorescence interferometry experiments are presented that measure macroscopic coherent kernels and their phase-relaxation in the low-temperature, bottom-state regime of the density-of-states below the migrational threshold energy where downhill site-to-site transfer is marginal. By using freely propagating and tunable 70 fs excitation/probing pulses and employing narrow-band spectral filtering of wave packets, fluorescence interferograms with strongly damped beatings can be observed. The coherences formally follow the in-phase superpositions of two site-optical free-induction-decays and originate from distinct pairs of coherent doorway-states, different in energy and space, each of them being targeted, by two discrete quantum-arrival-states 1α and 1β, via independent, isoenergetic 0→1 fluorescence transitions. The coherent transients are explained as site-to-site polarization beatings, caused by the interference of two fluorescence correlation signals. The numerical analysis of the damping regime, based upon second-order perturbational solutions, reveals the lower limit value of homogeneous dephasing in the range from T2≃100 fs to T2≃200 fs depending on the site-excitation energy of the bottom-states. The experiments enable to look into the formation of the relaxed state as a special molecular process of electron-phonon coupling and hence open-up a quite new perspective in the puzzle of multichromophore optical dynamics and structural relaxation in conjugated polymers.

  5. Optical control of molecular dynamics: Molecular cannons, reflectrons, and wave-packet focusers

    NASA Astrophysics Data System (ADS)

    Krause, Jeffrey L.; Whitnell, Robert M.; Wilson, Kent R.; Yan, YiJing; Mukamel, Shaul

    1993-11-01

    We consider the control of molecular dynamics using tailored light fields, based on a phase space theory of control [Y. J. Yan et al., J. Phys. Chem. 97, 2320 (1993)]. This theory enables us to calculate, in the weak field (one-photon) limit, the globally optimal light field that produces the best overlap for a given phase space target. We present as an illustrative example the use of quantum control to overcome the natural tendency of quantum wave packets to delocalize on excited state potential energy curves. Three cases are studied: (i) a ``molecular cannon'' in which we focus an outgoing continuum wave packet of I2 in both position and momentum, (ii) a ``reflectron'' in which we focus an incoming bound wave packet of I2, and (iii) the focusing of a bound wave packet of Na2 at a turning point on the excited state potential using multiple light pulses to create a localized wave packet with zero momentum. For each case, we compute the globally optimal light field and also how well the wave packet produced by this light field achieves the desired target. These globally optimal fields are quite simple and robust. While our theory provides the globally optimal light field in the linear, weak field regime, experiment can in reality only provide a restricted universe of possible light fields. We therefore also consider the control of molecular quantum dynamics using light fields restricted to a parametrized functional form which spans a set of fields that can be experimentally realized. We fit the globally optimal electric field with a functional form consisting of a superposition of subpulses with variable parameters of amplitude, center time, center frequency, temporal width, relative phase, and linear and quadratic chirp. The best fit light fields produce excellent quantum control and are within the range of experimental possibility. We discuss relevant experiments such as ultrafast spectroscopy and ultrafast electron and x-ray diffraction which can in principle

  6. Interferometry

    NASA Technical Reports Server (NTRS)

    Ridgway, Stephen; Wilson, Robert W.; Begelman, Mitchell C.; Bender, Peter; Burke, Bernard F.; Cornwell, Tim; Drever, Ronald; Dyck, H. Melvin; Johnston, Kenneth J.; Kibblewhite, Edward

    1991-01-01

    The following recommended programs are reviewed: (1) infrared and optical interferometry (a ground-based and space programs); (2) compensation for the atmosphere with adaptive optics (a program for development and implementation of adaptive optics); and (3) gravitational waves (high frequency gravitational wave sources (LIGO), low frequency gravitational wave sources (LAGOS), a gravitational wave observatory program, laser gravitational wave observatory in space, and technology development during the 1990's). Prospects for international collaboration and related issues are also discussed.

  7. Evolution of a wave packet scattered by a one-dimensional potential

    SciTech Connect

    Khachatrian, A Zh; Alexanyan, Al G; Khoetsyan, V A; Alexanyan, N A

    2013-06-30

    We consider the evolution of a wave packet that is made up of a group of the wave functions describing the stationary scattering process and tunnels through a one-dimensional potential of arbitrary form. As the main characteristics of the time difference of the tunnelling process, use is made of the propagation speed of the wave-packet maximum. We show that the known Hartman formula for the tunnelling time corresponds to the wave packet with a wavenumber-uniform spectral composition in the case, when the phase and transmission coefficient modulus dispersions are taken into account only in the linear approximation. The amplitude of the main peak of the transmitted wave intensity is proven to be independent of the tunnelling time and is determined by the transmission coefficient of the spectral component at the carrier frequency and the spectral width of the wave packet. In the limit of an infinitely wide potential barrier the amplitude of the wave-packet maximum is shown to tend to zero slower than the tunnelling time tends to its asymptotic value, i.e., indeed we deal with the paradox of an infinitely large propagation speed of a wave disturbance through the barrier. (propagation of wave fronts)

  8. Phase Structure of Strong-Field Tunneling Wave Packets from Molecules

    NASA Astrophysics Data System (ADS)

    Liu, Ming-Ming; Li, Min; Wu, Chengyin; Gong, Qihuang; Staudte, André; Liu, Yunquan

    2016-04-01

    We study the phase structure of the tunneling wave packets from strong-field ionization of molecules and present a molecular quantum-trajectory Monte Carlo model to describe the laser-driven dynamics of photoelectron momentum distributions of molecules. Using our model, we reproduce and explain the alignment-dependent molecular frame photoelectron spectra of strong-field tunneling ionization of N2 reported by M. Meckel et al. [Nat. Phys. 10, 594 (2014)]. In addition to modeling the low-energy photoelectron angular distributions quantitatively, we extract the phase structure of strong-field molecular tunneling wave packets, shedding light on its physical origin. The initial phase of the tunneling wave packets at the tunnel exit depends on both the initial transverse momentum distribution and the molecular internuclear distance. We further show that the ionizing molecular orbital has a critical effect on the initial phase of the tunneling wave packets. The phase structure of the photoelectron wave packet is a key ingredient for modeling strong-field molecular photoelectron holography, high-harmonic generation, and molecular orbital imaging.

  9. Higher order dispersion in the propagation of a gravity wave packet

    NASA Technical Reports Server (NTRS)

    Yeh, K. C.; Dong, B.

    1989-01-01

    To the first order of approximation, the complex amplitude of a wave packet in an anisotropic and dispersive medium is convected with the group of velocity. However, a gravity wave is a vector wave. Its wave packet must be formed by superposition of various wave numbers with corresponding frequencies, as is the case for scalar waves, and additionally by superposing many eigenmodes which also depend on the wave number. To represent the vector wave packet self-consistently, it is found that a gradient term must be included in the expansion. For a Guassian wave packet, this gradient term is shown to have important implications on the velocity vector as represented by its hodograph. Numerical results show that the hodograph is influenced by the location of the relative position of interest from the center of a Gaussian pulse. Higher order expansion shows that an initial Gaussian wave packet will retain its Gaussian shape as it propagates, but the pulse will spread in all directions with its major axis undergoing a rotation. Numerical results indicate that these higher order dispersive effects may be marginally observable in the atmosphere.

  10. Phase Structure of Strong-Field Tunneling Wave Packets from Molecules.

    PubMed

    Liu, Ming-Ming; Li, Min; Wu, Chengyin; Gong, Qihuang; Staudte, André; Liu, Yunquan

    2016-04-22

    We study the phase structure of the tunneling wave packets from strong-field ionization of molecules and present a molecular quantum-trajectory Monte Carlo model to describe the laser-driven dynamics of photoelectron momentum distributions of molecules. Using our model, we reproduce and explain the alignment-dependent molecular frame photoelectron spectra of strong-field tunneling ionization of N_{2} reported by M. Meckel et al. [Nat. Phys. 10, 594 (2014)]. In addition to modeling the low-energy photoelectron angular distributions quantitatively, we extract the phase structure of strong-field molecular tunneling wave packets, shedding light on its physical origin. The initial phase of the tunneling wave packets at the tunnel exit depends on both the initial transverse momentum distribution and the molecular internuclear distance. We further show that the ionizing molecular orbital has a critical effect on the initial phase of the tunneling wave packets. The phase structure of the photoelectron wave packet is a key ingredient for modeling strong-field molecular photoelectron holography, high-harmonic generation, and molecular orbital imaging. PMID:27152800

  11. Solitary waves in the resonant phenomenon between a surface gravity wave packet and an internal gravity wave

    NASA Technical Reports Server (NTRS)

    Sepulveda, Nicasio

    1987-01-01

    A two-layer inviscid incompressible fluid system of intermediate depth is considered. A multiple-scales perturbation technique is applied to the basic equations and boundary conditions for a two-layer fluid system to derive a system of weakly nonlinear partial integrodifferential equations governing the resonant interaction between a surface gravity wave packet and an internal gravity wave at an intermediate depth, providing a bridge between the existing shallow and deep fluid theories. The convolution integral term in these equations accounts for the dispersion in the lower-layer fluid. An iterative fast Fourier transform scheme is developed to find solitary wave solutions to this system of equations. The overtaking collision of two pairs of solitary waves, simulated using a spectral method, is found to be inelastic. It is found that the amplitude of the solitary waves changes slightly after the collision. The phase shifts these solitary waves undergo was calculated numerically.

  12. Analysis of wave packet motion in frequency and time domain: oxazine 1.

    PubMed

    Braun, Markus; Sobotta, Constanze; Dürr, Regina; Pulvermacher, Horst; Malkmus, Stephan

    2006-08-17

    Wave packet motion in the laser dye oxazine 1 in methanol is investigated by spectrally resolved transient absorption spectroscopy. The spectral range of 600-690 nm was accessible by amplified broadband probe pulses covering the overlap region of ground-state bleach and stimulated emission signal. The influence of vibrational wave packets on the optical signal is analyzed in the frequency domain and the time domain. For the analysis in the frequency domain an algorithm is presented that accounts for interference effects of neighbored vibrational modes. By this method amplitude, phase and decay time of vibrational modes are retrieved as a function of probe wavelength and distortions due to neighbored modes are reduced. The analysis of the data in the time domain yields complementary information on the intensity, central wavelength, and spectral width of the optical bleach spectrum due to wave packet motion. PMID:16898679

  13. Wave packet dynamics in various two-dimensional systems: A unified description

    SciTech Connect

    Singh, Ashutosh; Biswas, Tutul Ghosh, Tarun Kanti; Agarwal, Amit

    2015-03-15

    In this article we present an exact and unified description of wave packet dynamics in various 2D systems in the presence of a transverse magnetic field. We consider an initial minimum-uncertainty Gaussian wave packet and find that its long-term dynamics displays the universal phenomena of spontaneous collapse and quantum revival. We estimate the timescales associated with these phenomena based on very general arguments for various materials, whose carrier dynamics is described either by the Schrödinger equation or by the Dirac equation.

  14. Time delay of wave packets during their tunnelling through a quantum diode

    SciTech Connect

    Ivanov, N A; Skalozub, V V

    2014-04-28

    A modified saddle-point method is used to investigate the process of propagation of a wave packet through a quantum diode. A scattering matrix is constructed for the structure in question. The case of tunnelling of a packet with a Gaussian envelope through the diode is considered in detail. The time delay and the shape of the wave packet transmitted are calculated. The dependence of the delay time on the characteristics of the input packet and the internal characteristics of the quantum diode is studied. Possible applications of the results obtained are discussed. (laser applications and other topics in quantum electronics)

  15. Control of wave packets in lithium dimers with a state-selected pump-probe scheme

    NASA Astrophysics Data System (ADS)

    Dai, Xingcan

    A state-selected pump-probe scheme is used to control wave packet dynamics in Li2. In this scheme, a cw laser selects one electronic transition from the thermally populated ground state to the launch state A1Sigmau+ of Li2, from which an ultrashort pump pulse creates a superstition state on the electronic states of Li2 followed by another ultrashort pulse to excite the wave packet to the ground state of Li2+. Usually, an unperturbed level at the A1Sigmau+ state of Li2 is selected by the cw laser pulses. However, if the level of A1Sigmau+ is perturbed by b3piu, and then the wave packets that consist of the triplet states as well as the singlet states of Li2 are detected from the mixed levels. Since one of the triplet states is predissociative, the fast decay of the amplitudes of the wave packets that have the components of this predissociative state is observed. In order to study coherent multiphoton processes, Raman wave packets are created and manipulated with a pulse shaping system. The phase difference between the amplitude coefficients induced by resonant and off-resonant Raman transitions is shown directly by comparing the phases of the Raman wave packets excited by the resonant and off-resonant Raman transitions. The ionization processes employed in the probe step of the state-selective pump-probe scheme is fully explored in the second pulse shaping system in the path of the probe beam. It shows that the direct transitions from the electronic states involved in the wave packets are unlikely; while the autoionization and collision induced ionization from highly-excited Rydberg states are the main sources of the final ion signals. Some degree of the control of the wave packet dynamics is realized by shaping the probe pulses. The decoherence rates of quantum beats at the shelf region of the E1Sigma g+ state are measured to test theoretical results about pure dephasing rate in Li2. Finally, some schemes and preliminary results on physical realization of quantum

  16. Experimental observation of simultaneous wave and particle behavior in a narrowband single-photon wave packet

    NASA Astrophysics Data System (ADS)

    Yan, Hui; Liao, Kaiyu; Deng, Zhitao; He, Junyu; Xue, Zheng-Yuan; Zhang, Zhi-Ming; Zhu, Shi-Liang

    2015-04-01

    Light's wave-particle duality is at the heart of quantum mechanics and can be well illustrated by Wheeler's delayed-choice experiment: The choice of inserting or removing the second classical (quantum) beam splitter in a Mach-Zehnder interferometer determines the classical (quantum) wave-particle behavior of a photon. In this paper, we report our experiment on directly observing simultaneous wave and particle behavior in a narrowband single-photon wave packet by classically inserting or removing the second beam splitter when part of the wave packet passes through it. Our experiment demonstrates that the produced wave-particle state can be utilized in encoding quantum information.

  17. A Gaussian wave packet phase-space representation of quantum canonical statistics

    SciTech Connect

    Coughtrie, David J.; Tew, David P.

    2015-07-28

    We present a mapping of quantum canonical statistical averages onto a phase-space average over thawed Gaussian wave-packet (GWP) parameters, which is exact for harmonic systems at all temperatures. The mapping invokes an effective potential surface, experienced by the wave packets, and a temperature-dependent phase-space integrand, to correctly transition from the GWP average at low temperature to classical statistics at high temperature. Numerical tests on weakly and strongly anharmonic model systems demonstrate that thermal averages of the system energy and geometric properties are accurate to within 1% of the exact quantum values at all temperatures.

  18. Time-dependent treatment of scattering. II - Novel integral equation approach to quantum wave packets

    NASA Technical Reports Server (NTRS)

    Sharafeddin, Omar A.; Judson, Richard S.; Kouri, Donald J.; Hoffman, David K.

    1990-01-01

    The novel wave-packet propagation scheme presented is based on the time-dependent form of the Lippman-Schwinger integral equation and does not require extensive matrix inversions, thereby facilitating application to systems in which some degrees of freedom express the potential in a basis expansion. The matrix to be inverted is a function of the kinetic energy operator, and is accordingly diagonal in a Bessel function basis set. Transition amplitudes for various orbital angular momentum quantum numbers are obtainable via either Fourier transform of the amplitude density from the time to the energy domain, or the direct analysis of the scattered wave packet.

  19. Novel characterization of the nonlinear refractive response of materials using spatially and spectrally resolved interferometry

    NASA Astrophysics Data System (ADS)

    Meier, Amanda; Adams, Daniel; Squier, Jeff; Durfee, Charles

    2010-10-01

    Characterization of the nonlinear refractive index of a material is important in order to fully understand the nonlinear propagation of femtosecond laser pulses. The most common method to obtaining the nonlinear refractive index is Z-scan. However, since it averages over pulse duration and beam profile, Z-scan is not reliable when there is time- and intensity-dependence of the nonlinear response. The new method we are exploring to make these nonlinear refractive index measurements is spatially and spectrally resolved interferometry (SSRI). SSRI is a method that can give a simultaneous measurement of the spatial wave-front across the frequency or temporal profile of the pulse. The SSRI method proves better in measuring response at specific y and t, allowing it to measure both delayed response and saturation effects. The ability to make a measurement in both dimensions enables understanding of spatiotemporal dynamics in other experiments as cross-wave polarization and filamentation.

  20. The Many Faces of Ice and Nonlinear Interferometry

    NASA Astrophysics Data System (ADS)

    Shultz, Mary Jane

    Ice is likely the most ubiquitous solid in the Universe, yet even here on Earth its surface contains many mysteries. At atmospheric pressure, the stable form of ice is hexagonal ice; known as Ih. This contribution will present data about (i) equilibrium growth at the ice-water interface, (ii) procedures to generate any targeted ice face, and (iii) vibrational spectra of the ice-air interface. Contrary to common belief, the stable ice-water interfaces does not consist of the basal face; rather it consists of pyramidal or prism faces. Growth results from a balance between the molecular density and the top half-bilayer configuration. Arguments reminiscent of Pauling's residual entropy of ice generate the configurational contribution. Prism faces are favored due to greater entropy. Ice grows cryptomorphologically: the macroscopic sample does not reveal the crystalline axes. Locating the crystal axes as well as generating authentic faces for fundamental studies use a combination of the birefringence of ice and etch profiles. Surface vibrational spectroscopy supports an ice model consisting of extended, cooperative motion and beyond-bonding-partner determination of hydrogen bond strength. The surface vibrational spectrum is probed with the nonlinear spectroscopy sum frequency generation (SFG). Currently, nonlinearity limits use of SFG to diagnose interactions. This limitation can be circumvented by measuring the full, complex spectrum. We will report initial results from a newly invented nonlinear interferometer that reveals the full complex spectrum.

  1. Wave-packet dynamics of noninteracting ultracold bosons in an amplitude-modulated parabolic optical lattice

    NASA Astrophysics Data System (ADS)

    Yamakoshi, Tomotake; Watanabe, Shinichi

    2015-06-01

    The recent Aarhus experiment [Phys. Rev. A 88, 023620 (2013), 10.1103/PhysRevA.88.023620] produced wave packets by applying amplitude modulation to a trapped Bose-Einstein condensate (BEC) of 87Rb using an optical lattice. The present paper renders a theoretical account of this experimental production of wave packets and their subsequent time evolution, focusing on a one-dimensional noninteracting bosonic system as a fundamental starting point for accurate quantum analysis. Since experimental manipulation requires efficient wave-packet creation, we introduce the "single-Q Rabi model" to give a simple and reliable description of the interband transition. As a natural extension, we demonstrate enhancement of the wave-packet production by the "two-step Rabi oscillation method" using either one or two frequencies. The subsequent time evolution is affected by the intertwining of Bragg reflection and the Landau-Zener transition at each band gap, which is analyzed with the aid of a semiclassical theory [Phys. Rev. Lett. 110, 085302 (2013), 10.1103/PhysRevLett.110.085302].

  2. Nonperturbative quantum solutions to resonant four-wave mixing of two single-photon wave packets

    SciTech Connect

    Johnsson, Mattias; Fleischhauer, Michael

    2003-08-01

    We analyze both analytically and numerically the resonant four-wave mixing of two co-propagating single-photon wave packets. We present analytic expressions for the two-photon wave function, and show that quantum solutions exist which display a shape-preserving oscillatory exchange of excitations between the modes. Potential applications including quantum-information processing are discussed.

  3. Motion of an Electron Wave Packet in a Uniform Electric Field

    ERIC Educational Resources Information Center

    Churchill, John N.

    1978-01-01

    Energy eigenstates are superimposed in order to form a wave packet for an electron propagating in one dimension under the influence of a uniform, time-dependent electric field. A graphical method is presented by which one can obtain both the position and shape of the envelope. (BB)

  4. Tracking molecular wave packets in cesium dimers by coherent Raman scattering

    NASA Astrophysics Data System (ADS)

    Yuan, Luqi; Pestov, Dmitry; Murawski, Robert K.; Ariunbold, Gombojav O.; Zhi, Miaochan; Wang, Xi; Sautenkov, Vladimir A.; Rostovtsev, Yuri V.; Siebert, Torsten; Sokolov, Alexei V.

    2012-08-01

    We explore wave-packet dynamics in the ground X 1Σg+ and excited B 1Πu states of cesium dimers (Cs2). In particular, we study the dependence of the wave-packet dynamics on the relative timing between femtosecond pump, Stokes, and probe pulses in a nondegenerate BOXCARS beam geometry, which are commonly used for coherent anti-Stokes Raman scattering (CARS) spectroscopy. The experimental results are elucidated by theoretical calculations, which are based on the Liouville equations for the density matrix for the molecular states. We observe oscillations in CARS signals as functions of both Stokes and probe pulse delays with respect to the pump pulse. The oscillation period relates to the wave-packet motion cycle in either the ground or excited state of Cs2 molecules, depending on the sequence of the input laser pulses in time. The performed analysis can be applied to study and/or manipulate wave-packet dynamics in a variety of molecules. It also provides an excellent test platform for theoretical models of molecular systems.

  5. MHD nature of ionospheric wave packets generated by the solar terminator

    NASA Astrophysics Data System (ADS)

    Afraimovich, E. L.; Edemsky, I. K.; Voeykov, S. V.; Yasukevich, Yu. V.; Zhivetiev, I. V.

    2010-02-01

    The morphology of medium-scale traveling wave packets is for the first time presented based on the total electron content (TEC), measured at the global network of GPS receivers (up to 1500 stations) during the long period (from 1998 to 2007) and at the GPS/GEONET dense Japan network (1220 stations) in 2008—2009. In the time domain, these packets are chains of narrowband TEC variations (trains) with a duration of about 1—2 h, a total duration of up to 6 h, and a variation period of 10—30 min. In the winter Northern Hemisphere, traveling wave packets are observed mostly 3 h after the passage of the morning solar terminator. In the equinox they appear after the passage of the solar terminator without a pronounced delay or advance. In summer traveling wave packets are registered 1.5—2 h before the appearance of the evening solar terminator at the observation point when the solar terminator passes in the magnetically conjugate region. The spatial structure of traveling wave packets is characterized by a high degree of anisotropy and coherence at a distance larger than ten wavelengths (the wavelength is 100—300 km). A high quality of the oscillatory system and synchronization with the appearance of the solar terminator at the observation point and in the magnetically conjugate region indicate that the generation of traveling wave packets by the solar terminator is of the MHD nature. Our results for the first time experimentally confirm the hypothesis that the solar terminator generates ion sound waves, proposed by Huba et al. [2000b].

  6. Quantum dynamics of solid Ne upon photo-excitation of a NO impurity: A Gaussian wave packet approach

    SciTech Connect

    Unn-Toc, W.; Meier, C.; Halberstadt, N.; Uranga-Pina, Ll.; Rubayo-Soneira, J.

    2012-08-07

    A high-dimensional quantum wave packet approach based on Gaussian wave packets in Cartesian coordinates is presented. In this method, the high-dimensional wave packet is expressed as a product of time-dependent complex Gaussian functions, which describe the motion of individual atoms. It is applied to the ultrafast geometrical rearrangement dynamics of NO doped cryogenic Ne matrices after femtosecond laser pulse excitation. The static deformation of the solid due to the impurity as well as the dynamical response after femtosecond excitation are analyzed and compared to reduced dimensionality studies. The advantages and limitations of this method are analyzed in the perspective of future applications to other quantum solids.

  7. Spatiotemporal Imaging of Ultrafast Molecular Motion: Collapse and Revival of the D{sub 2}{sup +} Nuclear Wave Packet

    SciTech Connect

    Ergler, Th.; Rudenko, A.; Zrost, K.; Schroeter, C. D.; Moshammer, R.; Ullrich, J.; Feuerstein, B.

    2006-11-10

    We report on a real-time imaging of the ultrafast D{sub 2}{sup +} rovibrational nuclear wave-packet motion performed using a combination of a pump-probe setup with 7 fs laser pulses and a 'reaction-microscope' spectrometer. We observe fast dephasing (collapse) of the vibrational wave packet and its subsequent revival and prove rotational excitation in ultrashort laser pulses. Channel-selective Fourier analysis of the wave packet's long-term ({approx}3000 fs) evolution allows us to resolve its individual constituents, revealing unique information on the mechanisms of strong-field ionization and dissociation.

  8. Wave-packet treatment of reactor neutrino oscillation experiments and its implications on determining the neutrino mass hierarchy

    NASA Astrophysics Data System (ADS)

    Chan, Yat-Long; Chu, M.-C.; Tsui, Ka Ming; Wong, Chan Fai; Xu, Jianyi

    2016-06-01

    We derive the neutrino flavor transition probabilities with the neutrino treated as a wave packet. The decoherence and dispersion effects from the wave-packet treatment show up as damping and phase-shifting of the plane-wave neutrino oscillation patterns. If the energy uncertainty in the initial neutrino wave packet is larger than around 0.01 of the neutrino energy, the decoherence and dispersion effects would degrade the sensitivity of reactor neutrino experiments to mass hierarchy measurement to lower than 3 σ confidence level.

  9. Five-wave-packet linear optics quantum-error-correcting code

    SciTech Connect

    Walker, Thomas A.; Braunstein, Samuel L.

    2010-06-15

    In this article we outline a method for generating linear optics circuits that encode quantum-error-correcting codes. Using this method we produce a single-error-correcting code encoding one wave packet over five which can be implemented using linear optics and feed-forward correction. This code improves on the capacity of the best known code that can be implemented using linear optics and saturates the lower bound for the number of carriers needed for a single-error-correcting code. Our code can correct arbitrary single errors that occur randomly on each wave packet corresponding to a non-Gaussian error model, thus circumventing the so-called no-go theorem for Gaussian quantum-error correction.

  10. Wave packet dynamics of an atomic ion in a Paul trap

    NASA Astrophysics Data System (ADS)

    Hashemloo, A.; Dion, C. M.; Rahali, G.

    2016-07-01

    Using numerical simulations of the time-dependent Schrödinger equation, we study the full quantum dynamics of the motion of an atomic ion in a linear Paul trap. Such a trap is based on a time-varying, periodic electric field and hence corresponds to a time-dependent potential for the ion, which we model exactly. We compare the center-of-mass motion with that obtained from classical equations of motion, as well as to results based on a time-independent effective potential. We also study the oscillations of the width of the ion’s wave packet, including close to the border between stable (bounded) and unstable (unbounded) trajectories. Our results confirm that the center-of-mass motion always follows the classical trajectory, that the width of the wave packet is bounded for trapping within the stability region, and therefore that the classical trapping criterion is fully applicable to quantum motion.

  11. Reconstruction of an excited-state molecular wave packet with attosecond transient absorption spectroscopy

    NASA Astrophysics Data System (ADS)

    Cheng, Yan; Chini, Michael; Wang, Xiaowei; González-Castrillo, Alberto; Palacios, Alicia; Argenti, Luca; Martín, Fernando; Chang, Zenghu

    2016-08-01

    Attosecond science promises to allow new forms of quantum control in which a broadband isolated attosecond pulse excites a molecular wave packet consisting of a coherent superposition of multiple excited electronic states. This electronic excitation triggers nuclear motion on the molecular manifold of potential energy surfaces and can result in permanent rearrangement of the constituent atoms. Here, we demonstrate attosecond transient absorption spectroscopy (ATAS) as a viable probe of the electronic and nuclear dynamics initiated in excited states of a neutral molecule by a broadband vacuum ultraviolet pulse. Owing to the high spectral and temporal resolution of ATAS, we are able to reconstruct the time evolution of a vibrational wave packet within the excited B'Σ1u+ electronic state of H2 via the laser-perturbed transient absorption spectrum.

  12. Complex time dependent wave packet technique for thermal equilibrium systems - Electronic spectra

    NASA Technical Reports Server (NTRS)

    Reimers, J. R.; Wilson, K. R.; Heller, E. J.

    1983-01-01

    A time dependent wave packet method is presented for the rapid calculation of the properties of systems in thermal equilibrium and is applied, as an illustration, to electronic spectra. The thawed Gaussian approximation to quantum wave packet dynamics combined with evaluation of the density matrix operator by imaginary time propagation is shown to give exact electronic spectra for harmonic potentials and excellent results for both a Morse potential and for the band contours of the three transitions of the visible electronic absorption spectrum of the iodine molecule. The method, in principle, can be extended to many atoms (e.g., condensed phases) and to other properties (e.g., infrared and Raman spectra and thermodynamic variables).

  13. Wave packet revivals in a graphene quantum dot in a perpendicular magnetic field

    SciTech Connect

    Torres, J. J.

    2010-10-15

    We study the time evolution of localized wave packets in graphene quantum dots in a perpendicular magnetic field, focusing on the quasiclassical and revival periodicities, for different values of the magnetic field intensities in a theoretical framework. We have considered contributions of the two inequivalent points in the Brillouin zone. The revival time has been found as an observable that shows the break valley degeneracy.

  14. Flow patterns of rotating time-dependent Hartree-Fock wave packets

    NASA Astrophysics Data System (ADS)

    Rosina, M.; Bouten, M.; Van Leuven, P.

    1982-12-01

    A soluble model (Elliott's model in two dimensions) is used to study how well flow patterns and features of rotational motion are represented by the time-dependent Hartree-Fock approximation. Due to the spreading of the wave packet in the exact Schrödinger time-evolution, the agreement is good only for phenomena which probe the current during a short time interval.

  15. Extracting amplitudes for single and double ionization from a time-dependent wave packet

    SciTech Connect

    Palacios, A.; Rescigno, T. N.; McCurdy, C. W.

    2007-10-15

    A method is described for extracting double ionization amplitudes from a quantum wave packet for an atom after a short radiation pulse, but while the electrons are still interacting. The procedure involves the use of exterior complex scaling to effectively propagate the field-free solution to infinite times, and allows the use of existing integral formulas for double ionization amplitudes for two electron atoms and molecules.

  16. Quantum mechanical manifestation of cantori: Wave-packet localization in stochastic regions

    NASA Astrophysics Data System (ADS)

    Brown, Robert C.; Wyatt, Robert E.

    1986-07-01

    Numerical calculations for a model anharmonic system interacting with a laser are used to analyze the quantum mechanical implications of classical structure in stochastic regions due to cantori (associated with the breakup of invariant Kolmogorov-Arnol'd-Moser surfaces). The numerical results show that a quantum wave packet may remain localized, even though classical orbits are strongly chaotic. Consequently, the quantum dynamics continues to exhibit ``tunnelinglike'' behavior even when diffusion is not classically forbidden.

  17. Improving wave-packet revivals in circular billiards by applying constant magnetic fields

    SciTech Connect

    Delben, G. J.; Gusso, A.; Luz, M. G. E. da

    2006-05-15

    We show that the revivals structure of Gaussian wave packets for a charged particle with nonzero linear momentum placed in a circular billiard can be considerably improved by applying a perpendicular constant magnetic field of correct chosen intensity. To obtain the desired enhancement, the field must be turned on only at certain time values. We also briefly investigate how the shape of the evoluted packet at the revivals, with and without an external B, compares with the initial state.

  18. Measured photoemission from electron wave packets in a strong laser field.

    PubMed

    Ware, Michael; Cunningham, Eric; Coburn, Caleb; Peatross, Justin

    2016-02-15

    We present calibrated measurements of single-photon Thomson scattering from free electrons driven by a laser with intensity 1018  W/cm2. The measurements demonstrate that individual electrons radiate with the strength of point emitters, even when their wave packets spread to the scale of the driving-laser wavelength. The result agrees with predictions of quantum electrodynamics. PMID:26872164

  19. Observation of autoionization dynamics and sub-cycle quantum beating in electronic molecular wave packets

    NASA Astrophysics Data System (ADS)

    Reduzzi, M.; Chu, W.-C.; Feng, C.; Dubrouil, A.; Hummert, J.; Calegari, F.; Frassetto, F.; Poletto, L.; Kornilov, O.; Nisoli, M.; Lin, C.-D.; Sansone, G.

    2016-03-01

    The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds (T = 2.6 fs in the near infrared spectral range), an external optical field can induce changes in a medium on the sub-cycle timescale, i.e. in a few hundred attoseconds. In this work, we resolve the dynamics of autoionizing states on the femtosecond timescale and observe the sub-cycle evolution of a coherent electronic wave packet in a diatomic molecule, exploiting a tunable ultrashort extreme ultraviolet pulse and a synchronized infrared field. The experimental observations are based on measuring the variations of the extreme ultraviolet radiation transmitted through the molecular gas. The different mechanisms contributing to the wave packet dynamics are investigated through theoretical simulations and a simple three level model. The method is general and can be extended to the investigation of more complex systems.

  20. Initial dynamics of the Norrish Type I reaction in acetone: probing wave packet motion.

    PubMed

    Brogaard, Rasmus Y; Sølling, Theis I; Møller, Klaus B

    2011-02-10

    The Norrish Type I reaction in the S(1) (nπ*) state of acetone is a prototype case of ketone photochemistry. On the basis of results from time-resolved mass spectrometry (TRMS) and photoelectron spectroscopy (TRPES) experiments, it was recently suggested that after excitation the wave packet travels toward the S(1) minimum in less than 30 fs and stays there for more than 100 picoseconds [Chem. Phys. Lett.2008, 461, 193]. In this work we present simulated TRMS and TRPES signals based on ab initio multiple spawning simulations of the dynamics during the first 200 fs after excitation, getting quite good agreement with the experimental signals. We can explain the ultrafast decay of the experimental signals in the following manner: the wave packet simply travels, mainly along the deplanarization coordinate, out of the detection window of the ionizing probe. This window is so narrow that subsequent revival of the signal due to the coherent deplanarization vibration is not observed, meaning that from the point of view of the experiment the wave packets travels directly to the S(1) minimum. This result stresses the importance of pursuing a closer link to the experimental signal when using molecular dynamics simulations in interpreting experimental results. PMID:21229990

  1. Strong quantum violation of the gravitational weak equivalence principle by a non-Gaussian wave packet

    NASA Astrophysics Data System (ADS)

    Chowdhury, P.; Home, D.; Majumdar, A. S.; Mousavi, S. V.; Mozaffari, M. R.; Sinha, S.

    2012-01-01

    The weak equivalence principle of gravity is examined at the quantum level in two ways. First, the position detection probabilities of particles described by a non-Gaussian wave packet projected upwards against gravity around the classical turning point and also around the point of initial projection are calculated. These probabilities exhibit mass dependence at both these points, thereby reflecting the quantum violation of the weak equivalence principle. Second, the mean arrival time of freely falling particles is calculated using the quantum probability current, which also turns out to be mass dependent. Such a mass dependence is shown to be enhanced by increasing the non-Gaussianity parameter of the wave packet, thus signifying a stronger violation of the weak equivalence principle through a greater departure from Gaussianity of the initial wave packet. The mass dependence of both the position detection probabilities and the mean arrival time vanishes in the limit of large mass. Thus, compatibility between the weak equivalence principle and quantum mechanics is recovered in the macroscopic limit of the latter. A selection of Bohm trajectories is exhibited to illustrate these features in the free fall case.

  2. ACCELERATION OF THE SOLAR WIND BY ALFVEN WAVE PACKETS

    SciTech Connect

    Galinsky, V. L.; Shevchenko, V. I.

    2013-01-20

    A scale separation kinetic model of the solar wind acceleration is presented. The model assumes an isotropic Maxwellian distribution of protons and a constant influx of outward propagating Alfven waves with a single exponent Kolmogorov-type spectrum at the base of a coronal acceleration region ({approx}2 R {sub Sun }). Our results indicate that nonlinear cyclotron resonant interaction taking energy from Alfven waves and depositing it into mostly perpendicular heating of protons in initially weakly expanding plasma in a spherically non-uniform magnetic field is able to produce the typical fast solar wind velocities for the typical plasma and wave conditions after expansion to about 5-10 solar radii R {sub Sun }. The acceleration model takes into account the gravity force and the ambipolar electric field, as well as the mirror force, which plays the most important role in driving the solar wind acceleration. Contrary to the recent claims of Isenberg, the cold plasma dispersion only slightly slows down the acceleration and actually helps in obtaining the more realistic fast solar wind speeds.

  3. Numerical approximation of the Schrödinger equation with the electromagnetic field by the Hagedorn wave packets

    SciTech Connect

    Zhou, Zhennan

    2014-09-01

    In this paper, we approximate the semi-classical Schrödinger equation in the presence of electromagnetic field by the Hagedorn wave packets approach. By operator splitting, the Hamiltonian is divided into the modified part and the residual part. The modified Hamiltonian, which is the main new idea of this paper, is chosen by the fact that Hagedorn wave packets are localized both in space and momentum so that a crucial correction term is added to the truncated Hamiltonian, and is treated by evolving the parameters associated with the Hagedorn wave packets. The residual part is treated by a Galerkin approximation. We prove that, with the modified Hamiltonian only, the Hagedorn wave packets dynamics give the asymptotic solution with error O(ε{sup 1/2}), where ε is the scaled Planck constant. We also prove that, the Galerkin approximation for the residual Hamiltonian can reduce the approximation error to O(ε{sup k/2}), where k depends on the number of Hagedorn wave packets added to the dynamics. This approach is easy to implement, and can be naturally extended to the multidimensional cases. Unlike the high order Gaussian beam method, in which the non-constant cut-off function is necessary and some extra error is introduced, the Hagedorn wave packets approach gives a practical way to improve accuracy even when ε is not very small.

  4. Time-dependent wave packet averaged vibrational frequencies from femtosecond stimulated Raman spectra

    NASA Astrophysics Data System (ADS)

    Wu, Yue-Chao; Zhao, Bin; Lee, Soo-Y.

    2016-02-01

    Femtosecond stimulated Raman spectroscopy (FSRS) on the Stokes side arises from a third order polarization, P(3)(t), which is given by an overlap of a first order wave packet, |" separators=" Ψ2 ( 1 ) ( p u , t ) > , prepared by a narrow band (ps) Raman pump pulse, Epu(t), on the upper electronic e2 potential energy surface (PES), with a second order wave packet, <" separators=" Ψ1 ( 2 ) ( p r ∗ , p u , t ) | , that is prepared on the lower electronic e1 PES by a broadband (fs) probe pulse, Epr(t), acting on the first-order wave packet. In off-resonant FSRS, |" separators=" Ψ2 ( 1 ) ( p u , t ) > resembles the zeroth order wave packet |" separators=" Ψ1 ( 0 ) ( t ) > on the lower PES spatially, but with a force on |" separators=" Ψ2 ( 1 ) ( p u , t ) > along the coordinates of the reporter modes due to displacements in the equilibrium position, so that <" separators=" Ψ1 ( 2 ) ( p r ∗ , p u , t ) | will oscillate along those coordinates thus giving rise to similar oscillations in P(3)(t) with the frequencies of the reporter modes. So, by recovering P(3)(t) from the FSRS spectrum, we are able to deduce information on the time-dependent quantum-mechanical wave packet averaged frequencies, ω ¯ j ( t ) , of the reporter modes j along the trajectory of |" separators=" Ψ1 ( 0 ) ( t ) > . The observable FSRS Raman gain is related to the imaginary part of P(3)(ω). The imaginary and real parts of P(3)(ω) are related by the Kramers-Kronig relation. Hence, from the FSRS Raman gain, we can obtain the complex P(3)(ω), whose Fourier transform then gives us the complex P(3)(t) to analyze for ω ¯ j ( t ) . We apply the theory, first, to a two-dimensional model system with one conformational mode of low frequency and one reporter vibrational mode of higher frequency with good results, and then we apply it to the time-resolved FSRS spectra of the cis-trans isomerization of retinal in rhodopsin [P. Kukura et al., Science 310, 1006 (2005)]. We obtain the vibrational

  5. Confinement effects on an ultra-cold matter wave-packet by a square well impurity near the de-localization threshold: analytic solutions, scaling, and width properties

    NASA Astrophysics Data System (ADS)

    Méndez-Fragoso, Ricardo; Cabrera-Trujillo, Remigio

    2015-05-01

    The determination of the maximum number of atoms and the density profile of an ultra-cold wave-packet, under confinement conditions by an attractive impurity near the de-localization threshold, have been an open problem in ultra-cold atom physics. In this work, we study the effect of a wave-guide impurity on an ultra-cold matter wave-packet at the threshold of de-localization. The impurity is modeled by a 1-D square well potential with depth V 0 and length 2 R 0. Coupling of the square well potential to a contact impurity of strength β at the center is also considered. The time-independent non-linear Schrödinger equation describing a Bose-Einstein condensate at the delocalization threshold is exactly solved. The density profile, maximum non-linear coupling constant, g max, and maximum number of atoms, N max, prompt to be localized by the defect potential in the ground and first excited states are also reported. It is shown that g max and the density profiles become only functions of the reduced impurity size ξ = √ V 0 R 0. It is also found that the first excited state at the threshold of de-localization exists only for ξ ≥ π/(2√2), always holding a lower number of atoms than the corresponding ground state for the same reduced impurity size. Also, the addition of a repulsive contact impurity leads to a non-linear coupling constant at the de-localization threshold lower than that of the square well potential. In spite of the non-linear character of the Gross-Pitaevskii equation, it is found that a general scaling-law holds for defects with the same ξ, related with the same g max, having the same reduced density profile in the quasi-free direction. We report the full width at half maximum for the wave-function and density profile, finding a large spread for small reduced confining conditions. Implications of these results for the determination of the wave-packet properties under confinement in atom chip and Bose-Einstein condensates are presented with the

  6. Complex time paths for semiclassical wave packet propagation with complex trajectories

    NASA Astrophysics Data System (ADS)

    Petersen, Jakob; Kay, Kenneth G.

    2014-08-01

    The use of complex-valued trajectories in semiclassical wave packet methods can lead to problems that prevent calculation of the wave function in certain regions of the configuration space. We investigate this so-called bald spot problem in the context of generalized Gaussian wave packet dynamics. The analysis shows that the bald spot phenomenon is essentially due to the complex nature of the initial conditions for the trajectories. It is, therefore, expected to be a general feature of several semiclassical methods that rely on trajectories with such initial conditions. A bald region is created when a trajectory, needed to calculate the wave function at a given time, reaches a singularity of the potential energy function in the complex plane at an earlier, real time. This corresponds to passage of a branch point singularity across the real axis of the complex time plane. The missing portions of the wave function can be obtained by deforming the time path for the integration of the equations of motion into the complex plane so that the singularity is circumvented. We present examples of bald spots, singularity times, and suitable complex time paths for one-dimensional barrier transmission in the Eckart and Gaussian systems. Although the bald regions for the Eckart system are often localized, they are found to be semi-infinite for the Gaussian system. For the case of deep tunneling, the bald regions for both systems may encompass the entire portion of space occupied by the transmitted wave packet. Thus, the use of complex time paths becomes essential for a treatment of barrier tunneling.

  7. Effects of periodic kicking on dispersion and wave packet dynamics in graphene

    NASA Astrophysics Data System (ADS)

    Agarwala, Adhip; Bhattacharya, Utso; Dutta, Amit; Sen, Diptiman

    2016-05-01

    We study the effects of δ -function periodic kicks on the Floquet energy-momentum dispersion in graphene. We find that a rich variety of dispersions can appear depending on the parameters of the kicking: at certain points in the Brillouin zone, the dispersion can become linear but anisotropic, linear in one direction and quadratic in the perpendicular direction, gapped with a quadratic dispersion, or completely flat (called dynamical localization). We show all these results analytically and demonstrate them numerically through the dynamics of wave packets propagating in graphene. We propose experimental methods for producing these effects.

  8. The theory of magnetohydrodynamic wave generation by localized sources. II - Collisionless dissipation of wave packets

    NASA Technical Reports Server (NTRS)

    Collins, William

    1989-01-01

    The dispersion equation of Barnes (1966) is used to study the dissipation of asymptotic wave packets generated by localized periodic sources. The solutions of the equation are linear waves, damped by Landau and transit-time processes, in a collisionless warm plasma. For the case of an ideal MHD system, most of the waves emitted from a source are shown to cancel asympotically through destructive interference. The modes transporting significant flux to asymptotic distances are found to be Alfven waves and fast waves with theta (the angle between the magnetic field and the characteristics of the far-field waves) of about 0 and about pi/2.

  9. Tracking Autoionizing-Wave-Packet Dynamics at the 1-fs Temporal Scale

    NASA Astrophysics Data System (ADS)

    Skantzakis, E.; Tzallas, P.; Kruse, J. E.; Kalpouzos, C.; Faucher, O.; Tsakiris, G. D.; Charalambidis, D.

    2010-07-01

    We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ˜4eV are excited simultaneously. An XUV probe pulse tracks the oscillatory and decaying evolution of the formed wave packet. The Fourier transform of the measured trace reproduces the spectrum of the series. The present work paves the way for ultrabroadband XUV spectroscopy and studies of ultrafast dynamics in all states of matter.

  10. Time-reversal-symmetric single-photon wave packets for free-space quantum communication.

    PubMed

    Trautmann, N; Alber, G; Agarwal, G S; Leuchs, G

    2015-05-01

    Readout and retrieval processes are proposed for efficient, high-fidelity quantum state transfer between a matter qubit, encoded in the level structure of a single atom or ion, and a photonic qubit, encoded in a time-reversal-symmetric single-photon wave packet. They are based on controlling spontaneous photon emission and absorption of a matter qubit on demand in free space by stimulated Raman adiabatic passage. As these processes do not involve mode selection by high-finesse cavities or photon transport through optical fibers, they offer interesting perspectives as basic building blocks for free-space quantum-communication protocols. PMID:25978231

  11. Time-Reversal-Symmetric Single-Photon Wave Packets for Free-Space Quantum Communication

    NASA Astrophysics Data System (ADS)

    Trautmann, N.; Alber, G.; Agarwal, G. S.; Leuchs, G.

    2015-05-01

    Readout and retrieval processes are proposed for efficient, high-fidelity quantum state transfer between a matter qubit, encoded in the level structure of a single atom or ion, and a photonic qubit, encoded in a time-reversal-symmetric single-photon wave packet. They are based on controlling spontaneous photon emission and absorption of a matter qubit on demand in free space by stimulated Raman adiabatic passage. As these processes do not involve mode selection by high-finesse cavities or photon transport through optical fibers, they offer interesting perspectives as basic building blocks for free-space quantum-communication protocols.

  12. Steering the Electron in H{sub 2}{sup +} by Nuclear Wave Packet Dynamics

    SciTech Connect

    Fischer, Bettina; Kremer, Manuel; Pfeifer, Thomas; Feuerstein, Bernold; Sharma, Vandana; Schroeter, Claus Dieter; Moshammer, Robert; Ullrich, Joachim; Thumm, Uwe

    2010-11-26

    By combining carrier-envelope phase (CEP) stable light fields and the traditional method of optical pump-probe spectroscopy we study electron localization in dissociating H{sub 2}{sup +} molecular ions. Localization and localizability of electrons is observed to strongly depend on the time delay between the two CEP-stable laser pulses with a characteristic periodicity corresponding to the oscillating molecular wave packet. Variation of the pump-probe delay time allows us to uncover the underlying physical mechanism for electron localization, which are two distinct sets of interfering dissociation channels that exhibit specific temporal signatures in their asymmetry response.

  13. Wave-packet dynamics for general contact interactions on a circular setup: Revivals, bouncing, and trapping

    SciTech Connect

    Schmidt, Alexandre G.M.; Luz, M.G.E. da

    2004-05-01

    Here we study a one-dimensional finite lattice formed by generalized contact interactions in a circular setup, i.e., under periodic boundary conditions. Considering only four such potentials, we show the emergence of different behaviors as revivals, bouncing, and trapping for the time evolution of wave packets. This is done by properly choosing the parameters that characterize the contact interactions. We also discuss possible physical applications for this type of system, such as using it to split an initially localized state into spatially separated and dynamically independent parts.

  14. Fully differential study of wave packet scattering in ionization of helium by proton impact

    NASA Astrophysics Data System (ADS)

    Arthanayaka, T.; Lamichhane, B. R.; Hasan, A.; Gurung, S.; Remolina, J.; Borbély, S.; Járai-Szabó, F.; Nagy, L.; Schulz, M.

    2016-07-01

    We present a fully differential study of projectile coherence effects in ionization in p + He collisions. The experimental data are qualitatively reproduced by a non-perturbative ab initio time-dependent model, which treats the projectile coherence properties in terms of a wave packet. A comparison between first- and higher-order treatments shows that the observed interference structures are primarily due to a coherent superposition of different impact parameters leading to the same scattering angle. Higher-order contributions have a significant effect on the interference term.

  15. Three-Dimensional Momentum Imaging of Electron Wave Packet Interference in Few-Cycle Laser Pulses

    SciTech Connect

    Gopal, R.; Simeonidis, K.; Moshammer, R.; Ergler, Th.; Duerr, M.; Kurka, M.; Kuehnel, K.-U.; Tschuch, S.; Schroeter, C.-D.; Bauer, D.; Ullrich, J.; Rudenko, A.; Herrwerth, O.; Uphues, Th.; Schultze, M.; Goulielmakis, E.; Uiberacker, M.; Lezius, M.; Kling, M. F.

    2009-07-31

    Using a reaction microscope, three-dimensional (3D) electron (and ion) momentum (P) spectra have been recorded for carrier-envelope-phase (CEP) stabilized few-cycle (approx5 fs), intense (approx4x10{sup 14} W/cm{sup 2}) laser pulses (740 nm) impinging on He. Preferential emission of low-energy electrons (E{sub e}<15 eV) to either hemisphere is observed as a function of the CEP. Clear interference patterns emerge in P space at CEPs with maximum asymmetry, interpreted as attosecond interferences of rescattered and directly emitted electron wave packets by means of a simple model.

  16. The phase delay and its complex time: From stationary states up to wave packets

    SciTech Connect

    Grossel, Ph.

    2013-03-15

    Complex time is often invoked about tunneling effect where the classical phase delay is completed with a crucial filter effect. Usually the complex times are obtained by considering the flux-flux correlation function, but this can be obtained by a very simple approach using the search of the maximum of the generalized complex phase function, including the amplitude of the wave function. Various aspects of the phase delay are presented in the case of wave packets impinging on simple or resonant quantum barriers. Formal links with the classical mechanics give birth to quasi-trajectories of the quantum particle, totally compatible with the quantum mechanics. - Highlights: Black-Right-Pointing-Pointer The stationary phase method is extended in including the variations of the spectra. Black-Right-Pointing-Pointer The complex phase delay leads to a complex trajectory inside and out-side the barrier. Black-Right-Pointing-Pointer Examples of quasi-trajectories are given in case of different quantum barriers. Black-Right-Pointing-Pointer Phase delays are specified for resonant tunneling or above-barrier wave-packets. Black-Right-Pointing-Pointer The coherence between the quasi-trajectories and quantum mechanics is shown.

  17. Formation of two-dimensional nonspreading atomic wave packets in the field of two standing light waves

    SciTech Connect

    Efremov, M A; Fedorov, Mikhail V; Petropavlovsky, S V; Yakovlev, V P; Schleich, Wolfgang P

    2005-08-31

    The formation of two-dimensional nonspreading atomic wave packets produced in the interaction of a beam of two-level atoms with two standing light waves polarised in the same plane is considered. The mechanism providing a dispersionless particle dynamics is the balance of two processes: a rapid decay of the atomic wave function away from the field nodes due to spontaneous transitions to nonresonance states and the quantum broadening of the wave packets formed in the close vicinity of field nodes. Coordinate-dependent amplitudes and phases of the two-dimensional wave packets were found for the j{sub g}=0 {r_reversible} j{sub e}=1 transition. (fourth seminar to the memory of d.n. klyshko)

  18. Effects of the air pressure on the wave-packet dynamics of gaseous iodine molecules at room temperature

    NASA Astrophysics Data System (ADS)

    Fan, Rongwei; He, Ping; Chen, Deying; Xia, Yuanqin; Yu, Xin; Wang, Jialing; Jiang, Yugang

    2013-02-01

    Based on ultrafast laser pulses, time-resolved resonance enhancement coherent anti-Stokes Raman scattering (RE-CARS) is applied to investigate wave-packet dynamics in gaseous iodine. The effects of air pressure on the wave-packet dynamics of iodine molecules are studied at pressures ranging from 1.5 Torr to 750 Torr. The RE-CARS signals are recorded in a gas cell filled with a mixture of about 0.3 Torr iodine in air buffer gas at room temperature. The revivals and fractional revival structures in the wave-packet signal are found to gradually disappear with rising air pressure up to 750 Torr, and the decay behaviors of the excited B-state and ground X-state become faster with increasing air pressure, which is due to the collision effects of the molecules and the growing complexity of the spectra at high pressures.

  19. Phase and amplitude control in the formation and detection of rotational wave packets in the E 1Σg+ state of Li2

    NASA Astrophysics Data System (ADS)

    Uberna, Radoslaw; Khalil, Munira; Williams, Richard M.; Papanikolas, John M.; Leone, Stephen R.

    1998-06-01

    Femtosecond laser pulse amplitude/phase masking techniques are employed to control the formation and detection of rotational wave packets in the electronic E 1Σg+ state of lithium dimer. The wave packets are prepared by coherent excitation of rovibronic E 1Σg+(νE,JE) states of Li2 from a single intermediate state, A 1Σu+(νA=11,JA=28), and probed by time-resolved photoionization. In the detection step, the wave packet is projected onto the X 2Σg+ state of Li2+. New resonance structure in the X 2Σu+ ionic state continuum is obtained by measuring the wave packet signal modulation amplitude as a function of the frequencies removed from the spectrally dispersed probe pulse by insertion of a wire mask in a single-grating pulse shaper. A split glass phase mask inserted into the pulse shaper is used to produce step function changes in the spectral phase of the pulse. The phase relation among the wave packet states is varied by changing the relative phases of spectral components in the pump pulse and is monitored by measuring the changes in the phase of the rotational wave packet recurrences using an unmodified probe pulse. By altering the relative phases among the wave packet components, the spatial distribution of the initial wave packet probability density is varied, resulting in phase-dependent "alignment" of the probability density in angular space. Phase changes in the signal recurrences are also observed when a phase modified pulse is used in the wave packet detection step after wave packet preparation with an unmodified pulse. The formation and detection of the wave packets is discussed in terms of quantum interference between different excitation routes. The relative phase factors encoded in a single optical pulse (pump or probe) are transferred into the interference term of the measured signal through the molecule-photon interaction.

  20. Real-time observation of dynamics in rotational molecular wave packets by use of air-laser spectroscopy

    NASA Astrophysics Data System (ADS)

    Zeng, Bin; Chu, Wei; Li, Guihua; Yao, Jinping; Zhang, Haisu; Ni, Jielei; Jing, Chenrui; Xie, Hongqiang; Cheng, Ya

    2014-04-01

    Molecular rotational spectroscopy based on a strong-field-ionization-induced nitrogen laser is employed to investigate the time evolution of the rotational wave packet composed by a coherent superposition of quantum rotational states created in a field-free molecular alignment. We show that this technique uniquely allows real-time observation of the ultrafast dynamics of the molecular rotational wave packet. Our analysis also shows that there exist two channels of generation of the nitrogen laser, shedding light on the population inversion mechanism behind the air laser generated by intense femtosecond laser pulses.

  1. A wave packet model for electron transfer and its implications for the semiconductor-liquid interface

    SciTech Connect

    Smith, B.B.; Nozik, A.J.

    1999-11-11

    This paper establishes the computational feasibility and examines the implications of a particular technique for simulations of time dependent electron transfer (ET) at semiconductor-liquid interfaces (SLIs). The methodology uses a one electron formalism employing wave packets, pseudopotentials, and molecular dynamics, which the authors dub WPMD. They describe a detailed mechanism for SLI ET by using the methodology. The model is versatile enough to address conventional SLI ET, surface state and adsorption mediated ET, photoexcited ET, and ET between quantum dots and other microstructures. They contrast the perspectives of their WPMD model of SLI ET with those in traditional literature and find substantial differences. The use of standard Landau-Zener theory for SLI ET is found particularly problematic.

  2. Quantum dynamics of electronic transitions with Gauss-Hermite wave packets.

    PubMed

    Borrelli, Raffaele; Peluso, Andrea

    2016-03-21

    A new methodology based on the superposition of time-dependent Gauss-Hermite wave packets is developed to describe the wave function of a system in which several interacting electronic states are coupled to a bath of harmonic oscillators. The equations of motion for the wave function parameters are obtained by employing the Dirac-Frenkel time-dependent variational principle. The methodology is applied to study the quantum dynamical behaviour of model systems with two interacting electronic states characterized by a relatively large reorganization energy and a range of energy biases. The favourable scaling properties make it a promising tool for the study of the dynamics of chemico-physical processes in molecular systems. PMID:27004857

  3. A Gaussian Wave Packet Propagation Approach to Vibrationally Resolved Optical Spectra at Non-Zero Temperatures.

    PubMed

    Reddy, Ch Sridhar; Prasad, M Durga

    2016-04-28

    An effective time dependent approach based on a method that is similar to the Gaussian wave packet propagation (GWP) technique of Heller is developed for the computation of vibrationally resolved electronic spectra at finite temperatures in the harmonic, Franck-Condon/Hertzberg-Teller approximations. Since the vibrational thermal density matrix of the ground electronic surface and the time evolution operator on that surface commute, it is possible to write the spectrum generating correlation function as a trace of the time evolved doorway state. In the stated approximations, the doorway state is a superposition of the harmonic oscillator zero and one quantum eigenfunctions and thus can be propagated by the GWP. The algorithm has an O(N(3)) dependence on the number of vibrational modes. An application to pyrene absorption spectrum at two temperatures is presented as a proof of the concept. PMID:27035861

  4. Five-wave-packet quantum error correction based on continuous-variable cluster entanglement

    NASA Astrophysics Data System (ADS)

    Hao, Shuhong; Su, Xiaolong; Tian, Caixing; Xie, Changde; Peng, Kunchi

    2015-10-01

    Quantum error correction protects the quantum state against noise and decoherence in quantum communication and quantum computation, which enables one to perform fault-torrent quantum information processing. We experimentally demonstrate a quantum error correction scheme with a five-wave-packet code against a single stochastic error, the original theoretical model of which was firstly proposed by S. L. Braunstein and T. A. Walker. Five submodes of a continuous variable cluster entangled state of light are used for five encoding channels. Especially, in our encoding scheme the information of the input state is only distributed on three of the five channels and thus any error appearing in the remained two channels never affects the output state, i.e. the output quantum state is immune from the error in the two channels. The stochastic error on a single channel is corrected for both vacuum and squeezed input states and the achieved fidelities of the output states are beyond the corresponding classical limit.

  5. Probing the Spatial Structure of a Molecular Attosecond Electron Wave Packet Using Shaped Recollision Trajectories

    NASA Astrophysics Data System (ADS)

    Niikura, Hiromichi; Wörner, Hans Jakob; Villeneuve, D. M.; Corkum, P. B.

    2011-08-01

    Using orthogonally polarized 800 nm and 400 nm laser pulses, we have generated high harmonics in ethane (C2H6). We observe that the intensity of each harmonic order modulates with the attosecond delay between the two laser fields. The modulation period of the low even harmonics is twice that of the period of modulation of the other harmonics. By comparing with theoretical calculation, we show that the double periodicity is a result of the electron wave packet motion in the valence shell of C2H6 on the attosecond time-scale. Our method is a general approach to measuring internal electron dynamics which does not require molecular alignment, making it applicable to more complex molecules than previous approaches.

  6. Mechanisms of Auger-induced chemistry derived from wave packet dynamics.

    PubMed

    Su, Julius T; Goddard, William A

    2009-01-27

    To understand how core ionization and subsequent Auger decay lead to bond breaking in large systems, we simulate the wave packet dynamics of electrons in the hydrogenated diamond nanoparticle C(197)H(112). We find that surface core ionizations cause emission of carbon fragments and protons through a direct Auger mechanism, whereas deeper core ionizations cause hydrides to be emitted from the surface via remote heating, consistent with results from photon-stimulated desorption experiments [Hoffman A, Laikhtman A, (2006) J Phys Condens Mater 18:S1517-S1546]. This demonstrates that it is feasible to study the chemistry of highly excited large-scale systems using simulation and analysis tools comparable in simplicity to those used for classical molecular dynamics. PMID:19164568

  7. Time-of-Flight Measurements of Single-Electron Wave Packets in Quantum Hall Edge States

    NASA Astrophysics Data System (ADS)

    Kataoka, M.; Johnson, N.; Emary, C.; See, P.; Griffiths, J. P.; Jones, G. A. C.; Farrer, I.; Ritchie, D. A.; Pepper, M.; Janssen, T. J. B. M.

    2016-03-01

    We report time-of-flight measurements on electrons traveling in quantum Hall edge states. Hot-electron wave packets are emitted one per cycle into edge states formed along a depleted sample boundary. The electron arrival time is detected by driving a detector barrier with a square wave that acts as a shutter. By adding an extra path using a deflection barrier, we measure a delay in the arrival time, from which the edge-state velocity v is deduced. We find that v follows 1 /B dependence, in good agreement with the E →×B → drift. The edge potential is estimated from the energy dependence of v using a harmonic approximation.

  8. Goos-Haenchen shifts in frustrated total internal reflection studied with wave-packet propagation

    SciTech Connect

    Chen Xi; Li Chunfang; Wei Rongrong; Zhang Yan

    2009-07-15

    We have investigated the Goos-Haenchen (GH) shifts in frustrated total internal reflection (FTIR) studied with wave-packet propagation. In the first-order approximation of the transmission coefficient, the GH shift is exactly the expression given by a stationary phase method, thus saturating an asymptotic constant in two different ways depending on the angle of incidence. Taking the second-order approximation into account, the GH shift does not saturate with increasing gap width when the small beam size is used. The GH shift increases by decreasing the beamwidth at the small incidence angles, while for the large incidence angles it reveals a strong decrease by decreasing the beamwidth. These phenomena offer the better understanding of the GH shift and tunneling delay time in FTIR.

  9. Depth migration with Gaussian wave packets based on Poincaré wavelets

    NASA Astrophysics Data System (ADS)

    Gorodnitskiy, Evgeny; Perel, Maria; Geng, Yu; Wu, Ru-Shan

    2016-04-01

    An approach to depth migration, based on an integral representation of seismic data, that is, wavefields recorded on the boundary, is presented in terms of Poincaré wavelets. Each wavelet is taken as a boundary datum for a high-frequency asymptotic solution of the wave equation. This solution, which we call the quasiphoton or the Gaussian wave packet, decreases in a Gaussian manner away from a point running along a ray that is launched from the surface. The deformation of the propagating packet is taken into account in the migration algorithm. A numerical example of zero-offset migration with synthetic seismograms calculated for the 2-D SEG/EAGE salt model is presented. The result, which uses only 3.9 per cent of the total number of coefficients, is a satisfactory image, with a threshold of 0.75 per cent.

  10. Mechanisms of Auger-induced chemistry derived from wave packet dynamics

    PubMed Central

    Su, Julius T.; Goddard, William A.

    2009-01-01

    To understand how core ionization and subsequent Auger decay lead to bond breaking in large systems, we simulate the wave packet dynamics of electrons in the hydrogenated diamond nanoparticle C197H112. We find that surface core ionizations cause emission of carbon fragments and protons through a direct Auger mechanism, whereas deeper core ionizations cause hydrides to be emitted from the surface via remote heating, consistent with results from photon-stimulated desorption experiments [Hoffman A, Laikhtman A, (2006) J Phys Condens Mater 18:S1517–S1546]. This demonstrates that it is feasible to study the chemistry of highly excited large-scale systems using simulation and analysis tools comparable in simplicity to those used for classical molecular dynamics. PMID:19164568

  11. The stationary phase method for a wave packet in a semiconductor layered system. The applicability of the method

    NASA Astrophysics Data System (ADS)

    Rodríguez-Coppola, H.; Diago-Cisneros, L.; Pérez-Álvarez, R.

    2007-11-01

    Using the formal analysis made by Bohm [D. Bohm, Quantum Theory (Dover, New York, 1979)] to calculate approximately the phase time for a transmitted and the reflected wave packets through a potential barrier, we calculate the phase time for a semiconductor system formed by different mesoscopic layers. The transmitted and the reflected wave packets are analyzed and the applicability of this procedure, based on the stationary phase of a wave packet, is considered in different conditions. For the applicability of the stationary phase method an expression is obtained in the case of the transmitted wave depending only on the derivatives of the phase, up to third order. This condition indicates whether the parameters of the system allow us to define the wave packet by its leading term. The case of a multiple barrier systems is shown as an illustration of the results. This formalism includes the use of the transfer matrix to describe the central stratum, whether it is formed by one layer (the single barrier case), or two barriers and an inner well (the double barrier resonant tunneling semiconductor structure system), but one can assume that this stratum can be comprise of any number or any kind of semiconductor layers.

  12. Direct observation of isolated Damon-Eshbach and backward volume spin-wave packets in ferromagnetic microstripes.

    PubMed

    Wessels, Philipp; Vogel, Andreas; Tödt, Jan-Niklas; Wieland, Marek; Meier, Guido; Drescher, Markus

    2016-01-01

    The analysis of isolated spin-wave packets is crucial for the understanding of magnetic transport phenomena and is particularly interesting for applications in spintronic and magnonic devices, where isolated spin-wave packets implement an information processing scheme with negligible residual heat loss. We have captured microscale magnetization dynamics of single spin-wave packets in metallic ferromagnets in space and time. Using an optically driven high-current picosecond pulse source in combination with time-resolved scanning Kerr microscopy probed by femtosecond laser pulses, we demonstrate phase-sensitive real-space observation of spin-wave packets in confined permalloy (Ni80Fe20) microstripes. Impulsive excitation permits extraction of the dynamical parameters, i.e. phase- and group velocities, frequencies and wave vectors. In addition to well-established Damon-Eshbach modes our study reveals waves with counterpropagating group- and phase-velocities. Such unusual spin-wave motion is expected for backward volume modes where the phase fronts approach the excitation volume rather than emerging out of it due to the negative slope of the dispersion relation. These modes are difficult to excite and observe directly but feature analogies to negative refractive index materials, thus enabling model studies of wave propagation inside metamaterials. PMID:26906113

  13. Monitoring attosecond dynamics of coherent electron-nuclear wave packets by molecular high-order-harmonic generation

    SciTech Connect

    Bredtmann, Timm; Chelkowski, Szczepan; Bandrauk, Andre D.

    2011-08-15

    A pump-probe scheme for preparing and monitoring electron-nuclear motion in a dissociative coherent electron-nuclear wave packet is explored from numerical solutions of a non-Born-Oppenheimer time-dependent Schroedinger equation. A mid-ir intense few-cycle probe pulse is used to generate molecular high-order-harmonic generation (MHOHG) from a coherent superposition of two or more dissociative coherent electronic-nuclear wave packets, prepared by a femtosecond uv pump pulse. Varying the time delay between the intense ir probe pulse and the uv pump pulse by a few hundreds of attoseconds, the MHOHG signal intensity is shown to vary by orders of magnitude, thus showing the high sensitivity to electron-nuclear dynamics in coherent electron-nuclear wave packets. We relate this high sensitivity of MHOHG spectra to opposing electron velocities (fluxes) in the electron wave packets of the recombining (recolliding) ionized electron and of the bound electron in the initial coherent superposition of two electronic states.

  14. Wave packet dynamics for a system with position and time-dependent effective mass in an infinite square well

    SciTech Connect

    Vubangsi, M.; Tchoffo, M.; Fai, L. C.; Pisma’k, Yu. M.

    2015-12-15

    The problem of a particle with position and time-dependent effective mass in a one-dimensional infinite square well is treated by means of a quantum canonical formalism. The dynamics of a launched wave packet of the system reveals a peculiar revival pattern that is discussed. .

  15. Direct observation of isolated Damon-Eshbach and backward volume spin-wave packets in ferromagnetic microstripes

    PubMed Central

    Wessels, Philipp; Vogel, Andreas; Tödt, Jan-Niklas; Wieland, Marek; Meier, Guido; Drescher, Markus

    2016-01-01

    The analysis of isolated spin-wave packets is crucial for the understanding of magnetic transport phenomena and is particularly interesting for applications in spintronic and magnonic devices, where isolated spin-wave packets implement an information processing scheme with negligible residual heat loss. We have captured microscale magnetization dynamics of single spin-wave packets in metallic ferromagnets in space and time. Using an optically driven high-current picosecond pulse source in combination with time-resolved scanning Kerr microscopy probed by femtosecond laser pulses, we demonstrate phase-sensitive real-space observation of spin-wave packets in confined permalloy (Ni80Fe20) microstripes. Impulsive excitation permits extraction of the dynamical parameters, i.e. phase- and group velocities, frequencies and wave vectors. In addition to well-established Damon-Eshbach modes our study reveals waves with counterpropagating group- and phase-velocities. Such unusual spin-wave motion is expected for backward volume modes where the phase fronts approach the excitation volume rather than emerging out of it due to the negative slope of the dispersion relation. These modes are difficult to excite and observe directly but feature analogies to negative refractive index materials, thus enabling model studies of wave propagation inside metamaterials. PMID:26906113

  16. Direct observation of isolated Damon-Eshbach and backward volume spin-wave packets in ferromagnetic microstripes

    NASA Astrophysics Data System (ADS)

    Wessels, Philipp; Vogel, Andreas; Tödt, Jan-Niklas; Wieland, Marek; Meier, Guido; Drescher, Markus

    2016-02-01

    The analysis of isolated spin-wave packets is crucial for the understanding of magnetic transport phenomena and is particularly interesting for applications in spintronic and magnonic devices, where isolated spin-wave packets implement an information processing scheme with negligible residual heat loss. We have captured microscale magnetization dynamics of single spin-wave packets in metallic ferromagnets in space and time. Using an optically driven high-current picosecond pulse source in combination with time-resolved scanning Kerr microscopy probed by femtosecond laser pulses, we demonstrate phase-sensitive real-space observation of spin-wave packets in confined permalloy (Ni80Fe20) microstripes. Impulsive excitation permits extraction of the dynamical parameters, i.e. phase- and group velocities, frequencies and wave vectors. In addition to well-established Damon-Eshbach modes our study reveals waves with counterpropagating group- and phase-velocities. Such unusual spin-wave motion is expected for backward volume modes where the phase fronts approach the excitation volume rather than emerging out of it due to the negative slope of the dispersion relation. These modes are difficult to excite and observe directly but feature analogies to negative refractive index materials, thus enabling model studies of wave propagation inside metamaterials.

  17. Traveling Wave Packets of Total Electron Content Disturbances As Deduced From Global GPS Network Data

    NASA Astrophysics Data System (ADS)

    Afraimovich, E.; Lesyuta, O.; Lipko, Yu.; Perevalova, N.; Voyeikov, S.; Vodyannikov, V.; Yakovets, A.; Jacobi, Ch.

    This report discusses the experimental research results on the morphology and physi- cal origin of total electron content (TEC) pulsations as measured using the data from the global GPS network. Periodic electron density oscillations of the type of wave packets were investigated previously in terms of the hypothesis of their association with geomagnetic field (GP) pulsations. The greater part of evidence of the association between GP ad periodic electron density oscillations in the ionosphere was obtained by recording the frequency Doppler shift if the ionosphere-reflected radio signal and TEC variations measured using signals from geostationary satellites. However, many years of investigations have not yet provided thorough insight into the mechanisms ac- counting for the linkage between GP and ionospheric variations. One reason for that is the difficulty associated with obtaining statistically significant sets of experimental data. The use of the international ground-based network of two-frequency receivers of the navigation GPS system which comprised no less than 900 site as of August 2001 and is currently placing the data on the Internet, opens up a new era of a global, con- tinuous and fully computerized monitoring of ionospheric disturbances of a different class. This report presents a global morphology of TEC pulsations for 50 days with a different level of geomagnetic activity and the number of stations of the global GPS network from 100 to 300. A total number of the "receiver - GPS satellites" radio paths used in the analysis is about 500,000. Quasi-periodic TEC variations in the range of periods from 10 to 20 min are investigated, which is dictated by the fact that the data from the global GPS network are placed on the Internet with a standard temporal res- olution of 30 s. Most often, the observed TEC pulsations represent wave packets with a duration on the order of 1 hour. It was found that such TEC pulsations are a rela- tively rare event and are

  18. Influence of wave-packet dynamics on the medium gain of an atomic system

    SciTech Connect

    Delagnes, J. C.; Bouchene, M. A.

    2007-10-15

    A sequence of two femtosecond pulses--a strong driving {pi}-polarized pulse and a weak propagating {sigma}-polarized pulse--excites resonantly the S{sub 1/2}{yields}P{sub 1/2} transition of an atomic system. Strong interference effects take place in the system between absorption and emission paths leading to a substantial amplification of the {sigma} pulse. We study the influence of the fine structure on the medium gain when the contribution of the off-resonant P{sub 3/2} level is taken into account. A drastic reduction of the medium gain is obtained. This effect is explained within the bright-state-dark-state formalism where the strong driving pulse creates a wave packet that can be trapped in a state--the bright state--leading to a significant reduction of the gain for the {sigma} pulse. Finally, we also show that periodical gain dependence with the driving pulse energy exhibits a significant change in its period value (compared with expected Rabi oscillations)

  19. Dynamics of nuclear wave packets at the F center in alkali halides

    NASA Astrophysics Data System (ADS)

    Koyama, Takeshi; Suemoto, Tohru

    2011-07-01

    The F center in alkali halides is a well-known prototype of a strongly coupled localized electron-phonon system. This colour center is one of the long studied targets in the field of photophysics because it is simple but rich in variety. Steady-state spectroscopy, such as modulation spectroscopy and Raman scattering spectroscopy, has elucidated the strength of the electron-phonon coupling in the (meta-)stable state, i.e. the ground state and the relaxed excited state. Picosecond spectroscopy has improved understanding of the state mixing in the transient state. Owing to recent developments of ultrafast lasers with pulse widths shorter than oscillation periods of phonons, it has been possible to perform real-time observation of lattice vibration, and the understanding of the transient state has been remarkably expanded. In this paper, we review early and present studies on dynamics of electron-phonon coupling at the F center, especially recent real-time observations on the dynamics of nuclear wave packets in the excited state of the F center in KI, KBr, KCl and RbCl. These real-time observations reveal (i) spatial extension of the electronic wave function of a trapped electron, (ii) the difference between the coupled phonons in the ground state and the excited state, (iii) diabatic transition between the adiabatic potential energy surfaces and (iv) anharmonicity of the potential energy surface.

  20. Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets

    PubMed Central

    Pullen, M. G.; Wolter, B.; Le, A. -T.; Baudisch, M.; Sclafani, M.; Pires, H.; Schröter, C. D.; Ullrich, J.; Moshammer, R.; Pfeifer, T.; Lin, C. D.; Biegert, J.

    2016-01-01

    The ability to directly follow and time-resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser-induced electron diffraction can meet these requirements, it was recently concluded that molecules with particular orbital symmetries (such as πg) cannot be imaged using purely backscattering electron wave packets without molecular alignment. Here, we demonstrate, in direct contradiction to these findings, that the orientation and shape of molecular orbitals presents no impediment for retrieving molecular structure with adequate sampling of the momentum transfer space. We overcome previous issues by showcasing retrieval of the structure of randomly oriented O2 and C2H2 molecules, with πg and πu symmetries, respectively, and where their ionization probabilities do not maximize along their molecular axes. While this removes a serious bottleneck for laser-induced diffraction imaging, we find unexpectedly strong backscattering contributions from low-Z atoms. PMID:27329236

  1. Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets

    NASA Astrophysics Data System (ADS)

    Pullen, M. G.; Wolter, B.; Le, A.-T.; Baudisch, M.; Sclafani, M.; Pires, H.; Schröter, C. D.; Ullrich, J.; Moshammer, R.; Pfeifer, T.; Lin, C. D.; Biegert, J.

    2016-06-01

    The ability to directly follow and time-resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser-induced electron diffraction can meet these requirements, it was recently concluded that molecules with particular orbital symmetries (such as πg) cannot be imaged using purely backscattering electron wave packets without molecular alignment. Here, we demonstrate, in direct contradiction to these findings, that the orientation and shape of molecular orbitals presents no impediment for retrieving molecular structure with adequate sampling of the momentum transfer space. We overcome previous issues by showcasing retrieval of the structure of randomly oriented O2 and C2H2 molecules, with πg and πu symmetries, respectively, and where their ionization probabilities do not maximize along their molecular axes. While this removes a serious bottleneck for laser-induced diffraction imaging, we find unexpectedly strong backscattering contributions from low-Z atoms.

  2. Five-wave-packet quantum error correction based on continuous-variable cluster entanglement

    PubMed Central

    Hao, Shuhong; Su, Xiaolong; Tian, Caixing; Xie, Changde; Peng, Kunchi

    2015-01-01

    Quantum error correction protects the quantum state against noise and decoherence in quantum communication and quantum computation, which enables one to perform fault-torrent quantum information processing. We experimentally demonstrate a quantum error correction scheme with a five-wave-packet code against a single stochastic error, the original theoretical model of which was firstly proposed by S. L. Braunstein and T. A. Walker. Five submodes of a continuous variable cluster entangled state of light are used for five encoding channels. Especially, in our encoding scheme the information of the input state is only distributed on three of the five channels and thus any error appearing in the remained two channels never affects the output state, i.e. the output quantum state is immune from the error in the two channels. The stochastic error on a single channel is corrected for both vacuum and squeezed input states and the achieved fidelities of the output states are beyond the corresponding classical limit. PMID:26498395

  3. Effect of the disorder in graphene grain boundaries: A wave packet dynamics study

    NASA Astrophysics Data System (ADS)

    Vancsó, Péter; Márk, Géza I.; Lambin, Philippe; Mayer, Alexandre; Hwang, Chanyong; Biró, László P.

    2014-02-01

    Chemical vapor deposition (CVD) on Cu foil is one of the most promising methods to produce graphene samples despite of introducing numerous grain boundaries into the perfect graphene lattice. A rich variety of GB structures can be realized experimentally by controlling the parameters in the CVD method. Grain boundaries contain non-hexagonal carbon rings (4, 5, 7, 8 membered rings) and vacancies in various ratios and arrangements. Using wave packet dynamic (WPD) simulations and tight-binding electronic structure calculations, we have studied the effect of the structure of GBs on the transport properties. Three model GBs with increasing disorder were created in the computer: a periodic 5-7 GB, a "serpentine" GB, and a disordered GB containing 4, 8 membered rings and vacancies. It was found that for small energies (E = EF ± 1 eV) the transmission decreases with increasing disorder. Four membered rings and vacancies are identified as the principal scattering centers. Revealing the connection between the properties of GBs and the CVD growth method may open new opportunities in the graphene based nanoelectronics.

  4. Five-wave-packet quantum error correction based on continuous-variable cluster entanglement.

    PubMed

    Hao, Shuhong; Su, Xiaolong; Tian, Caixing; Xie, Changde; Peng, Kunchi

    2015-01-01

    Quantum error correction protects the quantum state against noise and decoherence in quantum communication and quantum computation, which enables one to perform fault-torrent quantum information processing. We experimentally demonstrate a quantum error correction scheme with a five-wave-packet code against a single stochastic error, the original theoretical model of which was firstly proposed by S. L. Braunstein and T. A. Walker. Five submodes of a continuous variable cluster entangled state of light are used for five encoding channels. Especially, in our encoding scheme the information of the input state is only distributed on three of the five channels and thus any error appearing in the remained two channels never affects the output state, i.e. the output quantum state is immune from the error in the two channels. The stochastic error on a single channel is corrected for both vacuum and squeezed input states and the achieved fidelities of the output states are beyond the corresponding classical limit. PMID:26498395

  5. On reduction of the wave-packet, decoherence, irreversibility and the second law of thermodynamics

    NASA Astrophysics Data System (ADS)

    Narnhofer, H.; Wreszinski, W. F.

    2014-08-01

    We prove a quantum version of the second law of thermodynamics: the (quantum) Boltzmann entropy increases if the initial (zero time) density matrix decoheres, a condition generally satisfied in Nature. It is illustrated by a model of wave-packet reduction, the Coleman-Hepp model, along the framework introduced by Sewell (2005) in his approach to the quantum measurement problem. Further models illustrate the monotonic-versus-non-monotonic behavior of the quantum Boltzmann entropy in time. As a last closely related topic, decoherence, which was shown by Narnhofer and Thirring (1999) to enforce macroscopic purity in the case of quantum K systems, is analyzed within a different class of quantum chaotic systems, viz. the quantum Anosov models as defined by Emch, Narnhofer, Sewell and Thirring (1994). A review of the concept of quantum Boltzmann entropy, as well as of some of the rigorous approaches to the quantum measurement problem within the framework of Schrödinger dynamics, is given, together with an overview of the C* algebra approach, which encompasses the relevant notions and definitions in a comprehensive way.

  6. Scattering of twisted particles: Extension to wave packets and orbital helicity

    NASA Astrophysics Data System (ADS)

    Ivanov, I. P.; Serbo, V. G.

    2011-09-01

    High-energy photons and other particles carrying nonzero orbital angular momentum (OAM) emerge as a new tool in high-energy physics. Recently, it was suggested to generate high-energy photons with nonzero OAM (twisted photons) by the Compton backscattering of twisted optical photons on relativistic electron beams. Twisted electrons in the intermediate energy range have also been demonstrated experimentally; twisted protons and other particles can, in principle, be created in a similar way. Collisions of energetic twisted states can offer a new look at particle properties and interactions. A theoretical description of twisted particle scattering developed previously treated them as pure Bessel states and ran into difficulty when describing the OAM of the final twisted particle at nonzero scattering angles. Here we develop further this formalism by incorporating two additional important features. First, we treat the initial OAM state as a wave packet of a finite transverse size rather than a pure Bessel state. This realistic assumption allows us to resolve the existing controversy between two theoretical analyses for nonforward scattering. Second, we describe the final twisted particle in terms of the orbital helicity: the OAM projection on its average direction of propagation rather than on the fixed reaction axis. Using this formalism, we determine to what extent the twisted state is transferred from the initial to final OAM particle in a generic scattering kinematics. As a particular application, we prove that in the Compton backscattering the orbital helicity of the final photon stays close to the OAM projection of the initial photon.

  7. Spatial-temporal control of interferences of multiple tunneling photoelectron wave packets

    NASA Astrophysics Data System (ADS)

    Li, Min; Geng, Ji-Wei; Liu, Ming-Ming; Zheng, Xu; Peng, Liang-You; Gong, Qihuang; Liu, Yunquan

    2015-07-01

    We theoretically study the control of the interferences of multiple tunneling photoelectron wave packets in both temporal and spatial domains by an orthogonally polarized two-color laser pulse. Profound carpetlike and stripelike interference patterns can be turned on or off in the momentum spectra using a weak streaking field at half the frequency of a strong fundamental field. The modulations of the interference patterns with respect to the relative phase between the two frequency components are well recaptured by both a semiclassical interference model and an ab initio simulation with numerically solving the time-dependent Schrödinger equation. We highlight the importance of the ionic Coulomb potential on the photoelectron angular distributions of atoms in the orthogonally polarized two-color pulses. It is shown that the interference induced by the forward rescattering trajectories is enhanced while the contribution of the direct trajectories is suppressed. This study offers alternative routes toward probing and controlling the ultrafast ionization dynamics of atoms and molecules.

  8. Wave-packet dynamical analysis of ultracold scattering in cylindrical waveguides

    SciTech Connect

    Melezhik, Vladimir S.; Kim, J. I.; Schmelcher, Peter

    2007-11-15

    A wave-packet propagation method is developed and applied to investigate the quantum dynamics of scattering processes of identical and distinguishable atoms in harmonic waveguides. The quantum dynamics of the confinement-induced resonances (CIRs) for ultracold collisions of identical particles, s-wave CIRs for bosons and p-wave CIRs for fermions, is explored in detail. Our multigrid approach allows us to fully take into account the coupling between the center-of-mass (c.m.) and relative motions in the case of distinguishable atoms. The latter includes, in particular, s- and p-partial-wave mixing, caused by the confining trap, which acts differently on the different atomic species. Specifically, we explore in detail the recently discovered [J. I. Kim, V. S. Melezhik, and P. Schmelcher, Phys. Rev. Lett. 97, 193203 (2006)] dual CIR, which is based on a destructive interference mechanism leading to complete transmission in the waveguide, although the corresponding scattering in free space exhibits strong s- and p-wave scattering.

  9. Semiclassical wave packet study of anomalous isotope effect in ozone formation.

    PubMed

    Vetoshkin, Evgeny; Babikov, Dmitri

    2007-10-21

    We applied the semiclassical initial value representation method to calculate energies, lifetimes, and wave functions of scattering resonances in a two-dimensional potential for O+O2 collision. Such scattering states represent the metastable O3* species and play a central role in the process of ozone formation. Autocorrelation functions for scattering states were computed and then analyzed using the Prony method, which permits one to extract accurate energies and widths of the resonances. We found that the results of the semiclassical wave packet propagation agree well with fully quantum results. The focus was on the 16O16O18O isotopomer and the anomalous isotope effect associated with formation of this molecule, either through the 16O16O+18O or the 16O+16O18O channels. An interesting correlation between the local vibration mode character of the metastable states and their lifetimes was observed and explained. New insight is obtained into the mechanism by which the long-lived resonances in the delta zero-point energy part of spectrum produce the anomalously large isotope effect. PMID:17949154

  10. Wave-packet continuum-discretization approach to ion-atom collisions: Nonrearrangement scattering

    NASA Astrophysics Data System (ADS)

    Abdurakhmanov, I. B.; Kadyrov, A. S.; Bray, I.

    2016-08-01

    A general single-center close-coupling approach based on a continuum-discretization procedure is developed to calculate excitation and ionization processes in ion-atom collisions. The continuous spectrum of the target is discretized using stationary wave packets constructed from the Coulomb wave functions, the eigenstates of the target Hamiltonian. Such continuum discretization allows one to generate pseudostates with arbitrary energies and distribution. These features are ideal for detailed differential ionization studies. The approach starts from the semiclassical three-body Schrödinger equation for the scattering wave function and leads to a set of coupled differential equations for the transition probability amplitudes. To demonstrate its utility the method is applied to calculate collisions of antiprotons with atomic hydrogen. A comprehensive set of benchmark results from integrated to fully differential cross sections for antiproton-impact ionization of hydrogen in the energy range from 1 keV to 1 MeV is provided. Contrary to previous predictions, we find that at low incident energies the singly differential cross section has a maximum away from the zero emission energy. This feature could not be seen without a fine discretization of the low-energy part of the continuum.

  11. Trojan Wave Packets in the Quantum Cavity within the Extended Jaynes-Cummings Model

    NASA Astrophysics Data System (ADS)

    Kalinski, Matt

    2016-05-01

    Some time ago we have developed the theory of the Trojan Wave Packets (TWP) in the classical strong Circularly Polarized electromagnetic field in terms of the Mathieu generating functions. We have discovered that by the proper partitioning of the Coulomb spectrum i.e. by considering the deviation from the circularity and the vertical tilt of the undressed states as the new quantum numbers we can reduce the problem to the problem of several non-interacting quantum pendula for the Stark-Zeeman field dressed states. The TWP in the infinite physical space however turned out to be weakly unstable due to the spontaneous emission. Here we develop the theory in which the TWP is truly eternal when the electromagnetic interactions are considered quantum and the field is confined by the perfect quantum cavity boundary conditions. First we extend the Jaynes-Cummings (JC) model from the two to the infinite number of levels interacting with the one or two perfectly resonant quantum modes of the electromagnetic field. Similarly the model of JC and our previous pendular model the dressed electron-field eigenstates are constructed within the weakly interacting manifolds. Superpositions of those states are possible with the quantum electron density moving on the circular trajectories.

  12. Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets

    DOE PAGESBeta

    Pullen, M. G.; Wolter, B.; Le, A. -T.; Baudisch, M.; Sclafani, M.; Pires, H.; Schroter, C. D.; Ullrich, J.; Moshammer, R.; Pfeifer, T.; et al

    2016-06-22

    The ability to directly follow and time-resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser-induced electron diffraction can meet these requirements, it was recently concluded that molecules with particular orbital symmetries (such as pg) cannot be imaged using purely backscattering electron wave packets without molecular alignment. Here, we demonstrate, in direct contradiction to these findings, that the orientation and shape of molecular orbitals presents no impediment for retrieving molecular structure with adequate sampling of the momentum transfer space. We overcome previous issues by showcasing retrieval ofmore » the structure of randomly oriented O2 and C2H2 molecules, with πg and πu symmetries, respectively, and where their ionization probabilities do not maximize along their molecular axes. As a result, while this removes a serious bottleneck for laser-induced diffraction imaging, we find unexpectedly strong backscattering contributions from low-Z atoms.« less

  13. Influence of orbital symmetry on diffraction imaging with rescattering electron wave packets.

    PubMed

    Pullen, M G; Wolter, B; Le, A-T; Baudisch, M; Sclafani, M; Pires, H; Schröter, C D; Ullrich, J; Moshammer, R; Pfeifer, T; Lin, C D; Biegert, J

    2016-01-01

    The ability to directly follow and time-resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser-induced electron diffraction can meet these requirements, it was recently concluded that molecules with particular orbital symmetries (such as πg) cannot be imaged using purely backscattering electron wave packets without molecular alignment. Here, we demonstrate, in direct contradiction to these findings, that the orientation and shape of molecular orbitals presents no impediment for retrieving molecular structure with adequate sampling of the momentum transfer space. We overcome previous issues by showcasing retrieval of the structure of randomly oriented O2 and C2H2 molecules, with πg and πu symmetries, respectively, and where their ionization probabilities do not maximize along their molecular axes. While this removes a serious bottleneck for laser-induced diffraction imaging, we find unexpectedly strong backscattering contributions from low-Z atoms. PMID:27329236

  14. Transient super-ballistic spreading of wave packets with large spreading exponents in some hybrid ordered-quasiperiodic lattices

    NASA Astrophysics Data System (ADS)

    Nguyen, Ba Phi; Ngo, Quang Minh; Kim, Kihong

    2016-02-01

    We consider the spreading of an initially localized wave packet in one-dimensional hybrid ordered-quasiperiodic lattices. We consider two diffrent kinds of quasiperiodic sequences, which are the Cantor and the period-doubling sequences. From numerical calculations based on the discrete Schrödinger equation, we demonstrate that hybrid ordered-quasiperiodic lattices can support the super-ballistic spreading of a wave packet with very large spreading exponents for certain transient time windows. Remarkably, in the case of the sublattice with the on-site potential obeying the period-doubling quasiperiodic sequence, we find that the super-ballistic exponent can be larger than six. We also point out that previous explanations of this phenomenon based on a generalized version of the point source model are incorrect.

  15. Dynamics of zero-energy nonspreading non-Gaussian wave packets for a class of central potentials

    SciTech Connect

    Makowski, Adam J. Pepłowski, Piotr

    2013-10-15

    Zero-energy wave packets, coherent states, are constructed in such a way that they retain their shape during the time evolution for a large class of central potentials. The packets are not of the Gaussian type with −r{sup 2} dependence but, instead, their shape is determined by −r{sup 1/(μ+1/2)} with −1/2<μ<1/2. A very close quantum–classical correspondence is also shown, i.e., the well localized states travel along suitable classical trajectories. -- Highlights: •Central potentials are considered. •Nonspreading, non-Gaussian wave packets are constructed. •Time evolution of the zero-energy packets is studied. •Quantum–classical correspondence is discussed.

  16. Coherent control of interfering wave packets in dissociating HD+ molecules: the role of phase and delay time

    NASA Astrophysics Data System (ADS)

    Qin, Chaochao; Zhang, Lili; Qiu, Xuejun; Zhang, Xianzhou; Liu, Yufang

    2016-02-01

    The coherent control of interference between dissociating wave packets of the HD+ molecules generated by a pair of time-delayed and phase-locked femtosecond laser pulses is theoretically studied by using the time-dependent quantum wave packet method. The density function in both coordinate and momentum representation are presented and discussed. It is demonstrated that the interference pattern is observed in both coordinate and momentum density functions. The interference undergoes a π-phase shift when the delay time between the two phase-locked femtosecond laser pulses is changed by half an optical period. In particular, the number of interference fringes, the fringe spacing in the R-dependent density distribution |ψ(R)|2, and the modulation period of the energy-dependent distribution of the fragments P(E) can be tuned by two phase-locked femtosecond pulses.

  17. Phase Coupling in Langmuir Wave Packets: Evidence for Four Wave Interactions in Solar Type III Radio Bursts

    NASA Technical Reports Server (NTRS)

    Thejappa, G.; MacDowall, R. J.; Bergamo, M.

    2012-01-01

    The four wave interaction process, known as the oscillating two stream instability (OTSI) is considered as one of the mechanisms responsible for stabilizing the electron beams associated with solar type III radio bursts. It has been reported that (1) an intense localized Langmuir wave packet associated with a type III burst contains the spectral characteristics of the OTSI: (a) a resonant peak at the local electron plasma frequency, f(sub pe), (b) a Stokes peak at a frequency slightly lower than f(sub pe), (c) anti-Stokes peak at a frequency slightly higher than f(sub pe), and (d) a low frequency enhancement below a few hundred Hz, (2) the frequencies and wave numbers of these spectral components satisfy the resonance conditions of the OTSI, and (3) the peak intensity of the wave packet is well above the thresholds for the OTSI as well as spatial collapse of envelope solitons. Here, for the first time, applying the trispectral analysis on this wave packet, we show that the tricoherence, which measures the degree of coherent four-wave coupling amongst the observed spectral components exhibits a peak. This provides an additional evidence for the OTSI and related spatial collapse of Langmuir envelope solitons in type III burst sources.

  18. Time dependent three-dimensional body frame quantal wave packet treatment of the H + H2 exchange reaction on the Liu-Siegbahn-Truhlar-Horowitz (LSTH) surface

    NASA Technical Reports Server (NTRS)

    Neuhauser, Daniel; Baer, Michael; Judson, Richard S.; Kouri, Donald J.

    1989-01-01

    The first successful application of the three-dimensional quantum body frame wave packet approach to reactive scattering is reported for the H + H2 exchange reaction on the LSTH potential surface. The method used is based on a procedure for calculating total reaction probabilities from wave packets. It is found that converged, vibrationally resolved reactive probabilities can be calculated with a grid that is not much larger than required for the pure inelastic calculation. Tabular results are presented for several energies.

  19. Time-dependent simulation and analytical modelling of electronic Mach-Zehnder interferometry with edge-states wave packets.

    PubMed

    Beggi, Andrea; Bordone, Paolo; Buscemi, Fabrizio; Bertoni, Andrea

    2015-12-01

    We compute the exact single-particle time-resolved dynamics of electronic Mach-Zehnder interferometers based on Landau edge-states transport, and assess the effect of the spatial localization of carriers on the interference pattern. The exact carrier dynamics is obtained by solving numerically the time-dependent Schrödinger equation with a suitable 2D potential profile reproducing the interferometer design. An external magnetic field, driving the system to the quantum Hall regime with filling factor one, is included. The injected carriers are represented by a superposition of edge states, and their interference pattern-controlled via magnetic field and/or area variation-reproduces the one of (Ji et al 2003 Nature 422 415). By tuning the system towards different regimes, we find two additional features in the transmission spectra, both related to carrier localization, namely a damping of the Aharonov-Bohm oscillations with increasing difference in the arms length, and an increased mean transmission that we trace to the energy-dependent transmittance of quantum point contacts. Finally, we present an analytical model, also accounting for the finite spatial dispersion of the carriers, able to reproduce the above effects. PMID:26548374

  20. Time-dependent simulation and analytical modelling of electronic Mach-Zehnder interferometry with edge-states wave packets

    NASA Astrophysics Data System (ADS)

    Beggi, Andrea; Bordone, Paolo; Buscemi, Fabrizio; Bertoni, Andrea

    2015-12-01

    We compute the exact single-particle time-resolved dynamics of electronic Mach-Zehnder interferometers based on Landau edge-states transport, and assess the effect of the spatial localization of carriers on the interference pattern. The exact carrier dynamics is obtained by solving numerically the time-dependent Schrödinger equation with a suitable 2D potential profile reproducing the interferometer design. An external magnetic field, driving the system to the quantum Hall regime with filling factor one, is included. The injected carriers are represented by a superposition of edge states, and their interference pattern—controlled via magnetic field and/or area variation—reproduces the one of (Ji et al 2003 Nature 422 415). By tuning the system towards different regimes, we find two additional features in the transmission spectra, both related to carrier localization, namely a damping of the Aharonov-Bohm oscillations with increasing difference in the arms length, and an increased mean transmission that we trace to the energy-dependent transmittance of quantum point contacts. Finally, we present an analytical model, also accounting for the finite spatial dispersion of the carriers, able to reproduce the above effects.

  1. Reconstruction and control of a time-dependent two-electron wave packet.

    PubMed

    Ott, Christian; Kaldun, Andreas; Argenti, Luca; Raith, Philipp; Meyer, Kristina; Laux, Martin; Zhang, Yizhu; Blättermann, Alexander; Hagstotz, Steffen; Ding, Thomas; Heck, Robert; Madroñero, Javier; Martín, Fernando; Pfeifer, Thomas

    2014-12-18

    The concerted motion of two or more bound electrons governs atomic and molecular non-equilibrium processes including chemical reactions, and hence there is much interest in developing a detailed understanding of such electron dynamics in the quantum regime. However, there is no exact solution for the quantum three-body problem, and as a result even the minimal system of two active electrons and a nucleus is analytically intractable. This makes experimental measurements of the dynamics of two bound and correlated electrons, as found in the helium atom, an attractive prospect. However, although the motion of single active electrons and holes has been observed with attosecond time resolution, comparable experiments on two-electron motion have so far remained out of reach. Here we show that a correlated two-electron wave packet can be reconstructed from a 1.2-femtosecond quantum beat among low-lying doubly excited states in helium. The beat appears in attosecond transient-absorption spectra measured with unprecedentedly high spectral resolution and in the presence of an intensity-tunable visible laser field. We tune the coupling between the two low-lying quantum states by adjusting the visible laser intensity, and use the Fano resonance as a phase-sensitive quantum interferometer to achieve coherent control of the two correlated electrons. Given the excellent agreement with large-scale quantum-mechanical calculations for the helium atom, we anticipate that multidimensional spectroscopy experiments of the type we report here will provide benchmark data for testing fundamental few-body quantum dynamics theory in more complex systems. They might also provide a route to the site-specific measurement and control of metastable electronic transition states that are at the heart of fundamental chemical reactions. PMID:25519135

  2. Spatio-temporal structure of the wave packets generated by the solar terminator

    NASA Astrophysics Data System (ADS)

    Afraimovich, E. L.; Edemskiy, I. K.; Voeykov, S. V.; Yasyukevich, Yu. V.; Zhivetiev, I. V.

    2009-10-01

    Using long-term (1998--2009) total electron content (TEC) measurements from the GPS global network including dense network of GPS sites in USA and Japan, we have obtained the first data regarding the spatio-temporal structure and the statistics of medium-scale traveling wave packets (MS TWPs) excited by the solar terminator (ST). Total amount of the detected TWPs exceeds 565,000. There is no correlation between TWPs occurrence and geomagnetic and solar activity. We found that the diurnal, seasonal and spectral MS TWPs characteristics are specified by the solar terminator (ST) dynamics. MS TWPs are the chains of narrow-band TEC oscillations with single packet's duration of about 1-2 h and oscillation periods of 10-20 min. The total duration of chain is about 4-6 h. The MS TWPs spatial structure is characterized by a high degree of anisotropy and coherence at the distance of more than 10 wavelengths. Occurrence rate of daytime MS TWPs is high in winter and during equinoxes. Occurrence rate of nighttime MS TWPs has its peak in summer. These features are consistent with previous MS travelling ionosphere disturbance (TID) statistics obtained from 630-nm airglow imaging observations in Japan. In winter, MS TWPs in the northern hemisphere are observed 3-4 h after the morning ST passage. In summer, MS TWPs are detected 1.5-2 h before the evening ST appearance at the point of observations, but at the moment of the evening ST passage in the magneto-conjugate point. The obtained results are the first experimental evidence for the hypothesis of the ST-generated ion sound waves.

  3. ‘Superluminal paradox’ in wave packet propagation and its quantum mechanical resolution

    SciTech Connect

    Sokolovski, D.; Akhmatskaya, E.

    2013-12-15

    We analyse in detail the reshaping mechanism leading to apparently ‘superluminal’ advancement of a wave packet traversing a classically forbidden region. In the coordinate representation, a barrier is shown to act as an effective beamsplitter, recombining envelopes of the freely propagating pulse with various spacial shifts. Causality ensures that none of the constituent envelopes are advanced with respect to free propagation, yet the resulting pulse is advanced due to a peculiar interference effect, similar to the one responsible for ‘anomalous’ values which occur in Aharonov’s ‘weak measurements’. In the momentum space, the effect is understood as a bandwidth phenomenon, where the incident pulse probes local, rather than global, analytical properties of the transmission amplitude T(p). The advancement is achieved when T(p) mimics locally an exponential behaviour, similar to the one occurring in Berry’s ‘superoscillations’. Seen in a broader quantum mechanical context, the ‘paradox’ is but a consequence of an attempt to obtain ‘which way?’ information without destroying the interference between the pathways of interest. This explains, to a large extent, the failure to adequately describe tunnelling in terms of a single ‘tunnelling time’. -- Highlights: •Apparent superluminality is described in the language of quantum measurements. •A barrier acts as a beamsplitter delaying copies of the initial pulse. •In the coordinate space the effect is similar to what occurs in ‘weak measurements’. •In the momentum space it relies on superoscillations in the transmission amplitude. •It is an interference effect, unlikely to be explained in simpler physical terms.

  4. Reconstruction and control of a time-dependent two-electron wave packet

    NASA Astrophysics Data System (ADS)

    Ott, Christian; Kaldun, Andreas; Argenti, Luca; Raith, Philipp; Meyer, Kristina; Laux, Martin; Zhang, Yizhu; Blättermann, Alexander; Hagstotz, Steffen; Ding, Thomas; Heck, Robert; Madroñero, Javier; Martín, Fernando; Pfeifer, Thomas

    2014-12-01

    The concerted motion of two or more bound electrons governs atomic and molecular non-equilibrium processes including chemical reactions, and hence there is much interest in developing a detailed understanding of such electron dynamics in the quantum regime. However, there is no exact solution for the quantum three-body problem, and as a result even the minimal system of two active electrons and a nucleus is analytically intractable. This makes experimental measurements of the dynamics of two bound and correlated electrons, as found in the helium atom, an attractive prospect. However, although the motion of single active electrons and holes has been observed with attosecond time resolution, comparable experiments on two-electron motion have so far remained out of reach. Here we show that a correlated two-electron wave packet can be reconstructed from a 1.2-femtosecond quantum beat among low-lying doubly excited states in helium. The beat appears in attosecond transient-absorption spectra measured with unprecedentedly high spectral resolution and in the presence of an intensity-tunable visible laser field. We tune the coupling between the two low-lying quantum states by adjusting the visible laser intensity, and use the Fano resonance as a phase-sensitive quantum interferometer to achieve coherent control of the two correlated electrons. Given the excellent agreement with large-scale quantum-mechanical calculations for the helium atom, we anticipate that multidimensional spectroscopy experiments of the type we report here will provide benchmark data for testing fundamental few-body quantum dynamics theory in more complex systems. They might also provide a route to the site-specific measurement and control of metastable electronic transition states that are at the heart of fundamental chemical reactions.

  5. Direct method for molecular wavepacket reconstruction on an unknown potential: Two-color nonlinear wavepacket interferometry on a photodissociative system

    NASA Astrophysics Data System (ADS)

    Humble, Travis S.; Cina, Jeffrey A.

    2003-03-01

    Nonlinear wavepacket interferometry (WPI) is a nonlinear optical technique that measures the contribution to molecular excited-state population that is quadrilinear in the electric fields of four femtosecond laser pulses comprising a pair of phase-locked pulse-pairs. The complex-valued overlap between one-pulse target and three-pulse reference vibrational wavepackets in an excited electronic state can be isolated from the nonlinear WPI signal by adding signals with different combinations of intrapulse-pair optical phase shifts. Using calculated WPI signals for a photodissociative model system of three electronic levels and nonzero pulse durations, we demonstrate that the set of isolable complex overlaps for a range of interpulse delays provides sufficient information to systematically reconstruct a time-dependent vibrational wavepacket prepared on an unknown potential by an unknown optical waveform. We apply our reconstruction procedure, based on singular-value decomposition in the position representation, to a shaped wavepacket prepared by linearly chirped pulses. The robustness of the reconstruction procedure is examined for various levels of signal noise and the presence of initial thermal population in multiple vibrational levels. It should be possible to incorporate nonlinear WPI measurements along the lines discussed here with closed-loop learning algorithms using existing pulse-shaping technology. In that context, the wavepacket reconstruction process could yield insights into the design and mechanism of action of shaped matter waves created by optimally crafted optical waveforms.

  6. Excitation of gravity waves by ocean surface wave packets: Upward propagation and reconstruction of the thermospheric gravity wave field

    NASA Astrophysics Data System (ADS)

    Vadas, Sharon L.; Makela, Jonathan J.; Nicolls, Michael J.; Milliff, Ralph F.

    2015-11-01

    In this paper, we derive the atmospheric gravity waves (GWs) and acoustic waves excited by an ocean surface wave packet with frequency ωF and duration χ in an f plane, isothermal, windless, and inviscid atmosphere. This packet is modeled as a localized vertical body force with Gaussian depth σz. The excited GW spectrum has discrete intrinsic frequencies (ωIr) at ωF and ωF±2π/χ ("sum" and "difference") and has a "continuum" of frequencies for ωIr<ωF+2π/χ. The momentum flux spectrum peaks at ωIr˜ωF and decreases rapidly as ωIr decreases. To simulate the effect these GWs have on the thermosphere, we present a new scheme whereby we sprinkle N GW spectra in the ocean wave packet region, ray trace the GWs, and reconstruct the GW field. We model the GWs excited by ocean wave packets with horizontal wavelengths of λH = 190 km, periods of τF = 2π/ωF = 14 - 20 min and χ = 30 - 50 min. The excited GWs begin to arrive at z = 250 km at t ˜ 75 - 80 min. Those with the largest temperature perturbations T' have large ωIr and arrive at t ˜ 90 - 130 min. If |α|=ωF+2π/χ is a solution of the GW dispersion relation and |α| is less than the buoyancy frequency at z = 250 km, the sum and highest-frequency continuum GWs have much larger phase speeds and arrive 50-60 min earlier with larger T' than the GWs with frequency ωF. For a packet with λH = 190 km, τF = 14 min, χ = 30 min, and height h0=1.3 m, the maximum T' at z = 250 km is ˜9, 22, and 40 K for σz = 1, 2, and 4 m, respectively.

  7. Quantum and semiclassical phase-space dynamics of a wave packet in strong fields using initial-value representations

    NASA Astrophysics Data System (ADS)

    Zagoya, C.; Wu, J.; Ronto, M.; Shalashilin, D. V.; Figueira de Morisson Faria, C.

    2014-10-01

    We assess the suitability of quantum and semiclassical initial-value representations (IVRs), exemplified by the coupled coherent states (CCS) method and the Herman-Kluk (HK) propagator, respectively, for modeling the dynamics of an electronic wave packet in a strong laser field, if this wave packet is initially bound. Using Wigner quasiprobability distributions and ensembles of classical trajectories, we identify signatures of over-the-barrier and tunnel ionization in phase space for static and time-dependent fields and the relevant sets of phase-space trajectories to model such features. Overall, we find good agreement with the full solution of the time-dependent Schrödinger equation (TDSE) for Wigner distributions constructed with both IVRs. Our results indicate that the HK propagator does not fully account for tunneling and over-the-barrier reflections. This leads to a dephasing in the time-dependent wave function, which becomes more pronounced for longer times. However, it is able to partly reproduce features associated with the wave packet crossing classically forbidden regions, although the trajectories employed in its construction always obey classical phase-space constraints. We also show that the CCS method represents a fully quantum initial value representation and accurately reproduces the results of a standard TDSE solver. Finally, we show that the HK propagator may be successfully employed to compute the time-dependent dipole acceleration and high-harmonic spectra. Nevertheless, the outcome of the semiclassical computation exhibits disagreements with the TDSE, as a consequence of the previously mentioned dephasing.

  8. Quantum state-to-state cross sections for atom-diatom reactions: A Chebyshev real wave-packet approach

    SciTech Connect

    Lin Shiying; Guo Hua

    2006-08-15

    We describe the implementation of a quantum mechanical method to calculate state-to-state differential cross sections for atom-diatom reactive scattering processes. The key ingredient of this approach is the efficient and accurate propagation of a real scattering wave packet in the Chebyshev order domain, from which the S-matrix elements can be extracted. This approach is implemented with Open MP and applied to compute differential and integral cross sections for the direct H+H{sub 2} abstraction reaction and the more challenging N({sup 2}D)+H{sub 2} insertion reaction.

  9. Real-Time Quadrature Measurement of a Single-Photon Wave Packet with Continuous Temporal-Mode Matching

    NASA Astrophysics Data System (ADS)

    Ogawa, Hisashi; Ohdan, Hideaki; Miyata, Kazunori; Taguchi, Masahiro; Makino, Kenzo; Yonezawa, Hidehiro; Yoshikawa, Jun-ichi; Furusawa, Akira

    2016-06-01

    Real-time controls based on quantum measurements are powerful tools for various quantum protocols. However, their experimental realization has been limited by mode mismatch between the temporal mode of quadrature measurement and that heralded by photon detection. Here, we demonstrate real-time quadrature measurement of a single-photon wave packet induced by photon detection by utilizing continuous temporal-mode matching between homodyne detection and an exponentially rising temporal mode. Single photons in exponentially rising modes are also expected to be useful resources for interactions with other quantum systems.

  10. Coherent and incoherent contributions to the carrier-envelope phase control of wave packet localization in quantum double wells

    SciTech Connect

    Hader, K.; Engel, V.

    2014-05-14

    We study laser excitation processes in a double well potential. The possibility to influence localization via the carrier-envelope phase (CEP) of a laser pulse is investigated for various situations which differ in the nature of the initial state prior to the laser interactions. In more detail, the CEP-dependence of asymmetries in the case where initially the system is described by localized wave packets, eigenstates, or incoherent mixtures are calculated and interpreted within time-dependent perturbation theory. It is investigated which contributions to the asymmetry exist and how they can be modified to reveal a more or less pronounced CEP-effect.

  11. Coherent electronic wave packet motion in C(60) controlled by the waveform and polarization of few-cycle laser fields.

    PubMed

    Li, H; Mignolet, B; Wachter, G; Skruszewicz, S; Zherebtsov, S; Süssmann, F; Kessel, A; Trushin, S A; Kling, Nora G; Kübel, M; Ahn, B; Kim, D; Ben-Itzhak, I; Cocke, C L; Fennel, T; Tiggesbäumker, J; Meiwes-Broer, K-H; Lemell, C; Burgdörfer, J; Levine, R D; Remacle, F; Kling, M F

    2015-03-27

    Strong laser fields can be used to trigger an ultrafast molecular response that involves electronic excitation and ionization dynamics. Here, we report on the experimental control of the spatial localization of the electronic excitation in the C_{60} fullerene exerted by an intense few-cycle (4 fs) pulse at 720 nm. The control is achieved by tailoring the carrier-envelope phase and the polarization of the laser pulse. We find that the maxima and minima of the photoemission-asymmetry parameter along the laser-polarization axis are synchronized with the localization of the coherent electronic wave packet at around the time of ionization. PMID:25860740

  12. Fusion reaction of halo nuclei: A real-time wave-packet method for three-body tunneling dynamics

    SciTech Connect

    Nakatsukasa, Takashi; Yabana, Kazuhiro; Ito, Makoto; Ueda, Manabu

    2006-08-14

    We investigate fusion cross section of a nucleus with a valence neutron, using the time-dependent wave-packet method. For a stable projectile, in which the valence neutron is tightly bound ({epsilon}n < -3 MeV), the neutron could enhance the fusion probability when the matching condition of orbital energies are satisfied. In contrast, for a halo nucleus, in which the binding energy of the neutron is very small ({epsilon}n > -1 MeV), the fusion probability is hindered by the presence of the weakly bound neutron.

  13. Overall non-linear correction of phase shifting mechanism in white light interferometry system based on displacement feedback control combined with fuzzy PID control

    NASA Astrophysics Data System (ADS)

    Song, Ningfang; Luo, Xinkai; Li, Huipeng; Li, Jiao

    2015-10-01

    The non-linearity of the phase shifting mechanism in white light interferometry system can seriously affect the measuring accuracy of the system. In this paper, the correcting method is to combine the displacement feedback control technology with the fuzzy PID control technology. Displacement feedback control mechanism and fuzzy PID controller are designed and then try to figure it out through Matlab simulation and experiment.. The result shows that combining the displacement feedback control technology with the fuzzy PID control technology can fulfill decent overall non-linear correction in the white light interferometry measuring system. Meanwhile, the accuracy of the correction is high and the non-linearity drop from 2% to 0.1%.

  14. Calculation of state-to-state differential and integral cross sections for atom-diatom reactions with transition-state wave packets

    SciTech Connect

    Zhao, Bin; Sun, Zhigang E-mail: hguo@unm.edu; Guo, Hua E-mail: hguo@unm.edu

    2014-06-21

    A recently proposed transition-state wave packet method [R. Welsch, F. Huarte-Larrañaga, and U. Manthe, J. Chem. Phys. 136, 064117 (2012)] provides an efficient and intuitive framework to study reactive quantum scattering at the state-to-state level. It propagates a few transition-state wave packets, defined by the eigenfunctions of the low-rank thermal flux operator located near the transition state, into the asymptotic regions of the reactant and product arrangement channels separately using the corresponding Jacobi coordinates. The entire S-matrix can then be assembled from the corresponding flux-flux cross-correlation functions for all arrangement channels. Since the transition-state wave packets can be defined in a relatively small region, its transformation into either the reactant or product Jacobi coordinates is accurate and efficient. Furthermore, the grid/basis for the propagation, including the maximum helicity quantum number K, is much smaller than that required in conventional wave packet treatments of state-to-state reactive scattering. This approach is implemented for atom-diatom reactions using a time-dependent wave packet method and applied to the H + D{sub 2} reaction with all partial waves. Excellent agreement with benchmark integral and differential cross sections is achieved.

  15. Dissipative Bohmian mechanics within the Caldirola–Kanai framework: A trajectory analysis of wave-packet dynamics in viscid media

    SciTech Connect

    Sanz, A.S.; Martínez-Casado, R.; Peñate-Rodríguez, H.C.; Rojas-Lorenzo, G.; Miret-Artés, S.

    2014-08-15

    Classical viscid media are quite common in our everyday life. However, we are not used to find such media in quantum mechanics, and much less to analyze their effects on the dynamics of quantum systems. In this regard, the Caldirola–Kanai time-dependent Hamiltonian constitutes an appealing model, accounting for friction without including environmental fluctuations (as it happens, for example, with quantum Brownian motion). Here, a Bohmian analysis of the associated friction dynamics is provided in order to understand how a hypothetical, purely quantum viscid medium would act on a wave packet from a (quantum) hydrodynamic viewpoint. To this purpose, a series of paradigmatic contexts have been chosen, such as the free particle, the motion under the action of a linear potential, the harmonic oscillator, or the superposition of two coherent wave packets. Apart from their analyticity, these examples illustrate interesting emerging behaviors, such as localization by “quantum freezing” or a particular type of quantum–classical correspondence. The reliability of the results analytically determined has been checked by means of numerical simulations, which has served to investigate other problems lacking of such analyticity (e.g., the coherent superpositions). - Highlights: • A dissipative Bohmian approach is developed within the Caldirola–Kanai model. • Some simple yet physically insightful systems are then studied analytically. • Dissipation leads to spatial localization in free-force regimes. • Under the action of linear forces, dissipation leads to uniform motion. • In harmonic potentials, the system decays unavoidable to the well minimum.

  16. Pairwise entanglement and readout of atomic-ensemble and optical wave-packet modes in traveling-wave Raman interactions

    SciTech Connect

    Wasilewski, Wojciech; Raymer, M. G.

    2006-06-15

    We analyze quantum entanglement of Stokes light and atomic electronic polarization excited during single-pass, linear-regime, stimulated Raman scattering in terms of optical wave-packet modes, and atomic-ensemble spatial modes. The output of this process is confirmed to be decomposable into multiple discrete, Bosonic mode pairs, each pair undergoing independent evolution into a two-mode squeezed state. For this we extend the Bloch-Messiah reduction theorem, previously known for discrete linear systems [S. L. Braunstein, Phys. Rev. A 71, 055801 (2005)]. We present typical mode functions in the case of one-dimensional scattering in an atomic vapor. We find that in the absence of dispersion, one mode pair dominates the process, leading to a simple interpretation of entanglement in this continuous-variable system. However, many mode pairs are excited in the presence of dispersion-induced temporal walkoff of the Stokes, as witnessed by the photon-count statistics. We also consider the readout of the stored atomic polarization using the anti-Stokes scattering process. We prove that the readout process can also be decomposed into multiple mode pairs, each pair undergoing independent evolution analogous to a beam-splitter transformation. We show that this process can have unit efficiency under realistic experimental conditions. The shape of the output light wave packet can be predicted. In the case of unit readout efficiency it contains only excitations originating from a specified atomic excitation mode.

  17. Quantum wave packet method for state-to-state reactive scattering calculations on AB + CD --> ABC + D reactions.

    PubMed

    Cvitas, Marko T; Althorpe, Stuart C

    2009-04-23

    We describe a quantum wave packet method for computing the state-to-state quantum dynamics of 4-atom AB + CD --> ABC + D reactions. The approach is an extension to 4-atom reactions of a version of the reactant-product decoupling (RPD) approach, applied previously to 3-atom reactions ( J. Chem. Phys. 2001, 114 , 1601 ). The approach partitions the coordinate space of the reaction into separate reagent, strong-interaction, and product regions, using a system of artificial absorbing and reflecting potentials. It employs a partitioned version of the split-operator propagator, which is more efficient than partitioning the (exact) time-dependent Schrodinger equation. The wave packet bounces off a reflecting potential in the entrance channel, which generates a source term; this is transformed efficiently from reagent to product Jacobi coordinates by exploiting some simple angular momentum properties. The efficiency and accuracy of the method is demonstrated by numerical tests on the benchmark OH + H(2) --> H(2)O + H reaction. PMID:19298045

  18. Dynamics of coupled plasmon polariton wave packets excited at a subwavelength slit in optically thin metal films

    NASA Astrophysics Data System (ADS)

    Wang, Lei-Ming; Zhang, Lingxiao; Seideman, Tamar; Petek, Hrvoje

    2012-10-01

    We study by numerical simulations the excitation and propagation dynamics of coupled surface plasmon polariton (SPP) wave packets (WPs) in optically thin Ag films and a bulk Ag/vacuum interface under the illumination of a subwavelength slit by 400 nm continuous wave (cw) and femtosecond pulsed light. The generated surface fields include contributions from both SPPs and quasicylindrical waves, which dominate in different regimes. We explore aspects of the coupled SPP modes in Ag thin films, including symmetry, propagation, attenuation, and the variation of coupling with incident angle and film thickness. Simulations of the electromagnetic transients initiated with femtosecond pulses reveal new features of coupled SPP WP generation and propagation in thin Ag films. Our results show that, under pulsed excitation, the SPP modes in an Ag thin film break up into two distinct bound surface wave packets characterized by marked differences in symmetries, group velocities, attenuation lengths, and dispersion properties. The nanometer spatial and femtosecond temporal scale excitation and propagation dynamics of the coupled SPP WPs are revealed in detail by movies recording the evolution of their transient field distributions.

  19. Time-resolved imaging of laser-induced vibrational wave packets in neutral and ionic states of iodomethane

    NASA Astrophysics Data System (ADS)

    Malakar, Y.; Kaderiya, B.; Zohrabi, M.; Pearson, W. L.; Ziaee, F.; Kananka Raju, P.; Ben-Itzhak, I.; Rolles, D.; Rudenko, A.

    2016-05-01

    Light-driven vibrational wave packets play an important role in molecular imaging and coherent control applications. Here we present the results of a pump-probe experiment characterizing laser-induced vibrational wave packets in both, neutral and ionic states of CH3 I (iodomethane), one of the prototypical polyatomic systems. Measuring yields and kinetic energies of all ionic fragments as a function of the time delay between two 25 fs, 800 nm pump and probe pulses, we map vibrational motion of the molecule, and identify the states involved by channel-resolved Fourier spectroscopy. In the Coulomb explosion channels we observe features with ~ 130 fs periodicity resulting from C-I symmetric stretch (ν3 mode) of the electronically excited cationic state. However the Fourier transform of the low-energy I+ ion yield produced by the dissociative ionization of CH3 I reveals the signatures of the same vibrational mode in the ground electronic states of both, neutral and cation, reflected in 65-70 fs oscillations. We observe the degeneration of the oscillatory structures from the cationic states within ~ 2 ps and discuss most likely reasons for this behavior. Supported by the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U. S. DOE. K. R. P. and W. L. P. supported by NSF Award No. IIA-143049.

  20. Time-dependent wave-packet method for the complete determination of S-matrix elements for reactive molecular collisions in three dimensions

    NASA Technical Reports Server (NTRS)

    Judson, Richard S.; Kouri, Donald J.; Neuhauser, Daniel; Baer, Michael

    1990-01-01

    An alternative time-dependent wave-packet method for treating three-dimensional gas phase reactive atom-diatom collisions is presented. The method employs a nonreactive body-frame wave packet propagation procedure, made possible by judicious use of absorbing optical potentials, a novel scheme for interpolating the wave function from coordinates in one arrangement to those in another and the fact that the time-dependent Schroedinger equation is an initial-value problem. The last feature makes possible a computationally viable and accurate procedure for changing from one arrangement's coordinates to another. In addition, the method allows the determination of S-matrix elements over a wide range of energies from a single wave-packet propagation. The method is illustrated by carrying out detailed calculations of inelastic and reactive scattering in the H + H2 system using the Liu-Siegbahn-Truhlar-Horowitz potential surface.

  1. Quantum wave packet study of nonadiabatic effects in O({sup 1}D) + H{sub 2} {yields} OH + H

    SciTech Connect

    Gray, S.K.; Petrongolo, C.; Drukker, K.; Schatz, G.C.

    1999-11-25

    The authors develop a wave packet approach to treating the electronically nonadiabatic reaction dynamics of O({sup 1}D) + H{sub 2} {yields} OH + H, allowing for the 1{sup 1}A{prime} and 2{sup 1}A{prime} potential energy surfaces and couplings, as well as the three internal nuclear coordinates. Two different systems of coupled potential energy surfaces are considered, a semiempirical diatomics-in-molecules (DIM) system due to Kuntz, Niefer, and Sloan, and a recently developed ab initio system due to Dobbyn and Knowles (DK). Nonadiabatic quantum results, with total angular momentum J = 0, are obtained and discussed. Several single surface calculations are carried out for comparison with the nonadiabatic results. Comparisons with trajectory surface hopping (TSH) calculations, and with approximate quantum calculations, are also included. The electrostatic coupling produces strong interactions between the 1{sup 1}A{prime} and 2{sup 1}A{prime} states at short range (where these states have a conical intersection) and weak but, interestingly, nonnegligible interactions between these states at longer range. The wave packet results show that if the initial state is chosen to be effectively the 1A{prime} state (for which insertion to form products occurs on the adiabatic surface), then there is very little difference between the adiabatic and coupled surface results. In either case the reaction probability is a relatively flat function of energy, except for resonant oscillations. However, the 2A{prime} reaction, dynamics (which involves a collinear transition state) is strongly perturbed by nonadiabatic effects in two distinct ways. At energies above the transition state barrier, the diabatic limit is dominant, and the 2A{prime} reaction probability is similar to that for 1A{double{underscore}prime}, which has no coupling with the other surfaces. At energies below the barrier, the authors find a significant component of the reaction probability from long range electronic

  2. PHYSICAL FOUNDATIONS OF QUANTUM ELECTRONICS: On the distortion of a wave packet propagating in an amplifying medium

    NASA Astrophysics Data System (ADS)

    Bukhman, N. S.

    2004-04-01

    The propagation of a narrow-band signal (wave packet) in a medium with population inversion is considered. It is shown that in an optically thick medium layer the signal decomposes into the initial and amplified signals propagating at different velocities and having different durations. The initial signal propagates without distortions at the velocity c/n0 (n0 is the refractive index of the medium away from the resonance frequency) and plays the role of a precursor of the amplified signal. The amplified signal moves at a lower velocity. It lags behind the initial signal during propagation and acquires a universal Gaussian shape (irrespective of the shape of the initial signal and the spectral line profile). The appearance of the amplified signal, which substantially differs from the initial signal in all the parameters, as well as the interference between the amplified and initial signals looks like a 'extra-distortion' of the initial signal.

  3. Dynamic Symmetry Breaking Hidden in Fano Resonance of a Molecule: S1 State of Diazirine Using Quantum Wave Packet Propagation.

    PubMed

    Park, Young Choon; An, Heesun; Lee, Yoon Sup; Baeck, Kyung Koo

    2016-02-18

    Fano resonance in the predissociation of the S1 state of diazirine was studied by applying a time-dependent wave packet propagation method, and dynamic symmetry breaking (DSB) around the stationary structure of S1 was disclosed in a detailed analysis of this theoretical result. The DSB was found to originate in coupling between the asymmetric C-N2 stretching and CH2 wagging modes, suggesting that there is a slight time gap between ring opening and the concurrent dragging of two H atoms of the CH2 moiety. Although the depth of the double well due to DSB is just 0.011 eV, its presence noticeably affects the early time dynamics and observed spectrum. PMID:26820379

  4. Simultaneous Observation of Wave Packet of the Atmospheric Gravity Waves by ISS-IMAP and All-sky Imager

    NASA Astrophysics Data System (ADS)

    Yukino, H.; Saito, A.; Sakanoi, T.; Otsuka, Y.

    2014-12-01

    The spatial scale of the atmospheric gravity wave in the mesosphere and the lower thermosphere was analyzed using the simultaneous observational data of ISS-IMAP and an all-sky imager at Hawaii. There are a plenty of previous studies that discuss the relationship between the wave structures of the mesospheric airglow and the tropospheric events. The problem of the ground-based observation of the airglow is that it cannot distinguish spatial variations from temporal variations for the structures whose scale size is larger than its field-of-view. ISS-IMAP started the observation in October, 2012 to survey the atmospheric gravity waves whose horizontal scale size is 50 km and longer. The spatial resolution of the VIsible-light and infrared Spectrum Imager (VISI) of ISS-IMAP/VISI imaging observation is from 10 km to 25 km. Simultaneous observations start from March 14, 2013. The atmospheric gravity waves that detected by VISI in 762 nm were compared with the observations of ground-based all-sky imagers in 557.7 nm. The generation and the propagation of the atmospheric gravity waves were investigated with this simultaneous observation. The relationship between the tropospheric events and the atmospheric gravity waves in the mesosphere is studied with the wide field-of-view observation by VISI/ISS-IMAP, and the continuous observation of the ground-based imagers. VISI frequently observed wave packets whose scale size is 1,000-2,000 km. These wave packets were observed by the ground-based imager as a series of waves whose wave length is 20-40 km, and that continue for 5-6 hours. The generation, the propagation and the distraction of the atmospheric gravity waves will be discussed in this presentation.

  5. Search for a nonlinear variant of the Schroedinger equation by neutron interferometry

    SciTech Connect

    Shull, C.G.; Atwood, D.K.; Arthur, J.; Horne, M.A.

    1980-03-24

    A slow-neutron interferometer system has been used to test a nonlinear variant of the Schroedinger equation ih partialpsi(r,t)/partialt=(-h/sup 2//2m)del/sup 2/+U(r,t))psi -b ln(a/sup 3/vertical-barpsivertical-bar/sup 2/)psi. If this equation were correct, then, as Shimony has suggested, repositioning an attenuating plate downstream in a neutron beam would produce a phase modification. No measurable phase shift beyond experimental uncertainty was found and an upper limit of 3.4 x 10/sup -13/ eV for the energy constant b was established.

  6. Nonlinear self-contraction of electron waves

    NASA Technical Reports Server (NTRS)

    Intrator, T.; Chan, C.; Hershkowitz, N.; Diebold, D.

    1984-01-01

    Laboratory evidence is presented of modulationally unstable electron wave packets which can be described by a nonlinear geometrical optics theory. Growth times for self-contraction are found to be much faster than ion response times and the bursts do not appear to be related to Zakharov Langmuir-wave collapse.

  7. Stability of two-dimensional ion-acoustic wave packets in quantum plasmas

    SciTech Connect

    Misra, A. P.; Marklund, M.; Brodin, G.; Shukla, P. K.

    2011-04-15

    The nonlinear propagation of two-dimensional (2D) quantum ion-acoustic waves (QIAWs) is studied in a quantum electron-ion plasma. By using a 2D quantum hydrodynamic model and the method of multiple scales, a new set of coupled nonlinear partial differential equations is derived which governs the slow modulation of the 2D QIAW packets. The oblique modulational instability (MI) is then studied by means of a corresponding nonlinear Schroedinger equation derived from the coupled nonlinear partial differential equations. It is shown that the quantum parameter H (ratio of the plasmon energy density to Fermi energy) shifts the MI domains around the k{theta} -plane, where k is the carrier wave number and {theta} is the angle of modulation. In particular, the ion-acoustic wave (IAW), previously known to be stable under parallel modulation in classical plasmas, is shown to be unstable in quantum plasmas. The growth rate of the MI is found to be quenched by the obliqueness of modulation. The modulation of 2D QIAW packets along the wave vector k is shown to be described by a set of Davey-Stewartson-like equations. The latter can be studied for the 2D wave collapse in dense plasmas. The predicted results, which could be important to look for stable wave propagation in laboratory experiments as well as in dense astrophysical plasmas, thus generalize the theory of MI of IAW propagations both in classical and quantum electron-ion plasmas.

  8. Combining 2D synchrosqueezed wave packet transform with optimization for crystal image analysis

    NASA Astrophysics Data System (ADS)

    Lu, Jianfeng; Wirth, Benedikt; Yang, Haizhao

    2016-04-01

    We develop a variational optimization method for crystal analysis in atomic resolution images, which uses information from a 2D synchrosqueezed transform (SST) as input. The synchrosqueezed transform is applied to extract initial information from atomic crystal images: crystal defects, rotations and the gradient of elastic deformation. The deformation gradient estimate is then improved outside the identified defect region via a variational approach, to obtain more robust results agreeing better with the physical constraints. The variational model is optimized by a nonlinear projected conjugate gradient method. Both examples of images from computer simulations and imaging experiments are analyzed, with results demonstrating the effectiveness of the proposed method.

  9. Instability of nonplanar modulated dust acoustic wave packets in a strongly coupled nonthermal dusty plasma

    SciTech Connect

    El-Labany, S. K. Zedan, N. A.; El-Taibany, W. F. E-mail: eltaibany@du.edu.eg

    2015-07-15

    Cylindrical and spherical amplitude modulations of dust acoustic (DA) solitary wave envelopes in a strongly coupled dusty plasma containing nonthermal distributed ions are studied. Employing a reductive perturbation technique, a modified nonlinear Schrödinger equation including the geometrical effect is derived. The influences of nonthermal ions, polarization force, and the geometries on the modulational instability conditions are analyzed and the possible rogue wave structures are discussed in detail. It is found that the spherical DA waves are more structurally stable to perturbations than the cylindrical ones. Possible applications of these theoretical findings are briefly discussed.

  10. Adjoint problem in duct acoustics and its reciprocity to forward problem by the Time Domain Wave Packet method

    NASA Astrophysics Data System (ADS)

    Kocaogul, Ibrahim; Hu, Fang; Li, Xiaodong

    2014-03-01

    Radiation of acoustic waves at all frequencies can be obtained by Time Domain Wave Packet (TDWP) method in a single time domain computation. Other benefit of the TDWP method is that it makes possible the separation of acoustic and instability wave in the shear flow. The TDWP method is also particularly useful for computations in the ducted or waveguide environments where incident wave modes can be imposed cleanly without a potentially long transient period. The adjoint equations for the linearized Euler equations are formulated for the Cartesian coordinates. Analytical solution for adjoint equations is derived by using Green's function in 2D and 3D. The derivation of reciprocal relations is presented for closed and open ducts. The adjoint equations are then solved numerically in reversed time by the TDWP method. Reciprocal relation between the duct mode amplitudes and far field point sources in the presence of the exhaust shear flow is computed and confirmed numerically. Applications of the adjoint problem to closed and open ducts are also presented.