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Sample records for polarized atomic photofragments

  1. An investigation of polarized atomic photofragments using the ion imaging technique

    SciTech Connect

    Bracker, A.S.

    1997-12-01

    This thesis describes measurement and analysis of the recoil angle dependence of atomic photofragment polarization (atomic v-J correlation). This property provides information on the electronic rearrangement which occurs during molecular photodissociation. Chapter 1 introduces concepts of photofragment vector correlations and reviews experimental and theoretical progress in this area. Chapter 2 described the photofragment ion imaging technique, which the author has used to study the atomic v-J correlation in chlorine and ozone dissociation. Chapter 3 outlines a method for isolating and describing the contribution to the image signal which is due exclusively to angular momentum alignment. Ion imaging results are presented and discussed in Chapter 4. Chapter 5 discusses a different set of experiments on the three-fragment dissociation of azomethane. 122 refs.

  2. Two-photon state selection and angular momentum polarization probed by velocity map imaging: application to H atom photofragment angular distributions from the photodissociation of two-photon state selected HCl and HBr.

    PubMed

    Manzhos, Sergei; Romanescu, Constantin; Loock, Hans-Peter; Underwood, Jonathan G

    2004-12-15

    A formalism for calculating the angular momentum polarization of an atom or a molecule following two-photon excitation of a J-selected state is presented. This formalism is used to interpret the H atom photofragment angular distributions from single-photon dissociation of two-photon rovibronically state selected HCl and HBr prepared via a Q-branch transition. By comparison of the angular distributions measured using the velocity map imaging technique with the theoretical model it is shown that single-photon dissociation of two-photon prepared states can be used for pathway identification, allowing for the identification of the virtual state symmetry in the two-photon absorption and/or the symmetry of the dissociative state. It is also shown that under conditions of excitation with circularly polarized light, or for excitation via non-Q-branch transitions with linearly polarized light the angular momentum polarization is independent of the dynamics of the two-photon transition and analytically computable. PMID:15634144

  3. The parity-adapted basis set in the formulation of the photofragment angular momentum polarization problem: The role of the Coriolis interaction

    SciTech Connect

    Shternin, Peter S.; Vasyutinskii, Oleg S.

    2008-05-21

    We present a theoretical framework for calculating the recoil-angle dependence of the photofragment angular momentum polarization taking into account both radial and Coriolis nonadiabatic interactions in the diatomic/linear photodissociating molecules. The parity-adapted representation of the total molecular wave function has been used throughout the paper. The obtained full quantum-mechanical expressions for the photofragment state multipoles have been simplified by using the semiclassical approximation in the high-J limit and then analyzed for the cases of direct photodissociation and slow predissociation in terms of the anisotropy parameters. In both cases, each anisotropy parameter can be presented as a linear combination of the generalized dynamical functions f{sub K}(q,q{sup '},q-tilde,q-tilde{sup '}) of the rank K representing contribution from different dissociation mechanisms including possible radial and Coriolis nonadiabatic transitions, coherent effects, and the rotation of the recoil axis. In the absence of the Coriolis interactions, the obtained results are equivalent to the earlier published ones. The angle-recoil dependence of the photofragment state multipoles for an arbitrary photolysis reaction is derived. As shown, the polarization of the photofragments in the photolysis of a diatomic or a polyatomic molecule can be described in terms of the anisotropy parameters irrespective of the photodissociation mechanism.

  4. Microfabricated Spin Polarized Atomic Magnetometers

    NASA Astrophysics Data System (ADS)

    Jimenez Martinez, Ricardo

    Spin polarized atomic magnetometers involve the preparation of atomic spins and their detection for monitoring magnetic fields. Due to the fact that magnetic fields are ubiquitous in our world, spin polarized atomic magnetometers are used in a wide range of applications from the detection of magnetic fields generated by the human heart and brain to the detection of nuclear magnetic resonance. In this thesis we developed microfabricated spin polarized atomic magnetometers. These sensors are based on optical pumping and spin-exchange collisions between alkali atoms and noble gases contained in microfabricated millimeter-scale vapor cells. In the first part of the thesis, we improved different features of current microfabricated optical magnetometers. Specifically, we improved the bandwidth of these devices, without degrading their magnetic field sensitivity, by broadening their magnetic resonance through spin-exchange collisions between alkali atoms. We also implemented all-optical excitation techniques to avoid problems, such as the magnetic perturbation of the environment, induced by the radio-frequency fields used in some of these sensors. In the second part of the thesis we demonstrated a microfluidic chip for the optical production and detection of hyperpolarized Xe gas through spin-exchange collisions with optically pumped Rb atoms. These devices are critical for the widespread use of spin polarized atomic magnetometers in applications requiring simple, compact, low-cost, and portable instrumentation.

  5. Molecular ion photofragment spectroscopy

    SciTech Connect

    Bustamente, S.W.

    1983-11-01

    A new molecular ion photofragment spectrometer is described which features a supersonic molecular beam ion source and a radio frequency octapole ion trap interaction region. This unique combination allows several techniques to be applied to the problem of detecting a photon absorption event of a molecular ion. In particular, it may be possible to obtain low resolution survey spectra of exotic molecular ions by using a direct vibrational predissociation process, or by using other more indirect detection methods. The use of the spectrometer is demonstrated by measuring the lifetime of the O/sub 2//sup +/(/sup 4/..pi../sub u/) metastable state which is found to consist of two main components: the /sup 4/..pi../sub 5/2/ and /sup 4/..pi../sub -1/2/ spin components having a long lifetime (approx. 129 ms) and the /sup 4/..pi../sub 3/2/ and /sup 4/..pi../sub 1/2/ spin components having a short lifetime (approx. 6 ms).

  6. Ionization of polarized hydrogen atoms

    SciTech Connect

    Alessi, J.G.

    1983-01-01

    Methods are discussed for the production of polarized H/sup -/ ions from polarized atoms produced in ground state atomic beam sources. Present day sources use ionizers of two basic types - electron ionizers for H/sup +/ Vector production followed by double charge exchange in a vapor, or direct H/sup -/ Vector production by charge exchange of H/sup 0/ with Cs/sup 0/. Both methods have ionization efficiencies of less than 0.5%. Ionization efficiencies in excess of 10% may be obtained in the future by the use of a plasma ionizer plus charge exchange in Cs or Sr vapor, or ionization by resonant charge exchange with a self-extracted D/sup -/ beam from a ring magnetron or HCD source. 36 references, 4 figures.

  7. Communication: Angular momentum alignment and fluorescence polarization of alkali atoms photodetached from helium nanodroplets

    SciTech Connect

    Hernando, Alberto; Beswick, J. Alberto; Halberstadt, Nadine

    2013-12-14

    The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms produced is calculated quantum mechanically by solving the excited states coupled equations with potentials determined by density functional theory (DFT). Pronounced oscillations as a function of excitation energy are predicted for the case of Na@(He){sub 200}, in marked contrast with the absorption cross-section and angular distribution of the ejected atoms which are smooth functions of the energy. These oscillations are due to quantum interference between different coherently excited photodetachment pathways. Experimentally, these oscillations should be reflected in the fluorescence polarization and polarization-resolved photoelectron yield of the ejected atoms, which are proportional to the electronic angular momentum alignment. In addition, this result is much more general than the test case of NaHe{sub 200} studied here. It should be observable for larger droplets, for higher excited electronic states, and for other alkali as well as for alkali-earth atoms. Detection of these oscillations would show that the widely used pseudo-diatomic model can be valid beyond the prediction of absorption spectra and could help in interpreting parts of the dynamics, as already hinted by some experimental results on angular anisotropy of bare alkali fragments.

  8. Communication: angular momentum alignment and fluorescence polarization of alkali atoms photodetached from helium nanodroplets.

    PubMed

    Hernando, Alberto; Beswick, J Alberto; Halberstadt, Nadine

    2013-12-14

    The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms produced is calculated quantum mechanically by solving the excited states coupled equations with potentials determined by density functional theory (DFT). Pronounced oscillations as a function of excitation energy are predicted for the case of Na@(He)200, in marked contrast with the absorption cross-section and angular distribution of the ejected atoms which are smooth functions of the energy. These oscillations are due to quantum interference between different coherently excited photodetachment pathways. Experimentally, these oscillations should be reflected in the fluorescence polarization and polarization-resolved photoelectron yield of the ejected atoms, which are proportional to the electronic angular momentum alignment. In addition, this result is much more general than the test case of NaHe200 studied here. It should be observable for larger droplets, for higher excited electronic states, and for other alkali as well as for alkali-earth atoms. Detection of these oscillations would show that the widely used pseudo-diatomic model can be valid beyond the prediction of absorption spectra and could help in interpreting parts of the dynamics, as already hinted by some experimental results on angular anisotropy of bare alkali fragments. PMID:24329048

  9. Polarization phenomena in multiphoton ionization of atoms

    NASA Technical Reports Server (NTRS)

    Jacobs, V. L.

    1973-01-01

    The theory of multiphoton ionization for an atomic system of arbitrary complexity is developed using a density matrix formalism. An expression is obtained which determines the differential N-photon ionization cross section as a function of the polarization states of the target atom and the incident radiation. The parameters which characterize the photoelectron angular distribution are related to the general reduced matrix elements for the N-photon transition. Two-photon ionization of unpolarized atoms is treated as an illustration of the use of the theory. The dependence of the multiphoton ionization cross section on the polarization state of the incident radiation, which has been observed in two- and three-photon ionization of Cs, is accounted for by the theory. Finally, the photoelectron spin polarization produced by the multiphoton ionization of unpolarized atoms, like the analogous polarization resulting from single-photon ionization, is found to depend on the circular polarization of the incident radiation.

  10. Assembling Ultracold Polar Molecules From Single Atoms

    NASA Astrophysics Data System (ADS)

    Liu, Lee R.; Hutzler, Nicholas R.; Yu, Yichao; Zhang, Jessie T.; Ni, Kang-Kuen

    2016-05-01

    Ultracold polar molecules are promising candidates for studying quantum many-body phenomena and building quantum information systems, due to their long-range, anisotropic, and tunable interactions. This calls for a technique to create low entropy samples of ultracold polar molecules with a large dipole moment. The lowest entropy molecular gas to date was created from atomic quantum gases in bulk or in optical lattices. The entropy is limited by that of the constituent atomic gases. We propose a method that addresses this limitation by assembling sodium cesium (NaCs) molecules from individually manipulated atoms. First, we load single Na and Cs atoms in separate optical tweezers from MOTs. We will cool them to their motional ground state using Raman sideband cooling and then merge them into a single tweezer. The tweezer confinement provides enhanced wavefunction overlap between the atom pair and molecule states. Using coherent two-photon techniques, we will then transfer the atom pair into a molecule. Our method offers reduced apparatus complexity and cycle time, single-site manipulation and imaging resolution, and should be readily extended to different species.

  11. The physics of spin polarized atomic vapors

    NASA Astrophysics Data System (ADS)

    Happer, William

    1988-05-01

    Research efforts are focussed on the study of spin polarized atoms, nuclei and electrons during the period covered by this report. Although this work is 6.1 basic research, it has applications to a number of important Air Force problems. For example, the atomic clocks used on the GPS satellite system operate with optically pumped rubidium absorption cells, very similar to the ones being investigated here. A number of the scientists and engineers working on atomic clocks used by Air Force satellite systems were trained with the support of this grant. We have participated in recent Air Force advisory panels to review concepts for high-energy-density fuels based on spin polarized atoms and molecules. The insights gained from research sponsored by this grant have been very useful in evaluating these ideas. Recent work has focussed on two main areas, the investigation of quadrupolar interactions between spin polarized noble gas nuclei and surfaces and the quantitative investigation of how magnetic field inhomogeneities cause spin relaxation.

  12. Ultrafast charge transfer and atomic orbital polarization

    SciTech Connect

    Deppe, M.; Foehlisch, A.; Hennies, F.; Nagasono, M.; Beye, M.; Sanchez-Portal, D.; Echenique, P. M.; Wurth, W.

    2007-11-07

    The role of orbital polarization for ultrafast charge transfer between an atomic adsorbate and a substrate is explored. Core hole clock spectroscopy with linearly polarized x-ray radiation allows to selectively excite adsorbate resonance states with defined spatial orientation relative to the substrate surface. For c(4x2)S/Ru(0001) the charge transfer times between the sulfur 2s{sup -1}3p*{sup +1} antibonding resonance and the ruthenium substrate have been studied, with the 2s electron excited into the 3p{sub perpendicular}* state along the surface normal and the 3p{sub parallel}* state in the surface plane. The charge transfer times are determined as 0.18{+-}0.07 and 0.84{+-}0.23 fs, respectively. This variation is the direct consequence of the different adsorbate-substrate orbital overlap.

  13. Photofragment imaging: The photo-dissociation of bromomethane, bromoethane, and bromoethanol

    SciTech Connect

    Chandler, D.W. ); Thoman, J.W. Jr. . Dept. of Chemistry); Hess, W.P. )

    1990-09-01

    Bromomethane, bromoethane and bromoethanol are photolyzed with 205-nm light and the velocity of the bromine atoms is recorded by the technique of photofragment imaging. The velocity distribution of the bromine atoms is a direct reflection of the internal-state distribution of the methyl, ethyl, and hydroxy-ethyl radicals and the orientation of the transition moment in the parent molecule. 8 refs., 2 figs., 1 tab.

  14. The HERMES Polarized Atomic Beam Source

    SciTech Connect

    Nass, A.

    2003-07-30

    The atomic beam source (ABS) provides nuclear polarized hydrogen or deuterium atoms for the HERMES target at flow rates of about 6.5 {center_dot} 1016H-vector/s (hydrogen in two hyperfine substates) and 6.0 {center_dot} 1016D-vector/s (deuterium in three hyperfine substates). The degree of dissociation of 93% for H (95% for D) at the entrance of the storage cell and the nuclear polarization of around 0.97 (H) and 0.92 (D) have been found to be constant within a a couple of percent over the whole running period of the HERMES experiment. A new dissociator (MWD) based on a microwave discharge at 2.45 GHz has been developed and installed into the HERMES-ABS in 2000. Since the velocity distribution of the MWD differs from that of the RFD the intensity could be increased further with a modified sextupole magnet system. For this purpose the way for a new start generator for sextupole tracking calculations was opened. Monte-Carlo simulations were successfully used to describe the gas expansion between nozzle, skimmer and collimator. A new type of beam monitor was used to study the beam formation after the nozzle.

  15. Atomic nitrogen densities near the polar cusp

    NASA Technical Reports Server (NTRS)

    Engebretson, M. J.; Nelson, J. T.

    1986-01-01

    The neutral atmospheric composition spectrometer on board the Dynamics Explorer 2 spacecraft sampled several major and minor thermospheric gases including atomic nitrogen. A selection of passes over the polar cusp that provide a quantitative measure of N densities in this region and provide evidence of localized density increases due to soft particle precipitation is presented. Increases in N densities are frequently observed but are smaller than accompanying increases in N2 densities. The observations support earlier studies suggesting that N densities increase more rapidly than O densities during periods of high solar EUV flux and N densities are larger in the summer hemisphere than in the winter hemisphere. A series of passes in February 1983, late in the lifetime of DE 2, indicated N densities at 200 km altitude were a factor of 2 larger near the southern cusp than near the northern cusp.

  16. Atomic nitrogen densities near the polar cusp

    NASA Technical Reports Server (NTRS)

    Engebretson, M. J.; Nelson, J. T.

    1985-01-01

    The neutral atmospheric composition spectrometer on board the Dynamics Explorer 2 spacecraft sampled several major and minor thermospheric gases including atomic nitrogen. A selection of passes over the polar cusp that provide a quantitative measure of N densities in this region and provide evidence of localized density increases due to soft particle precipitation is presented. Increases in N densities are frequently observed but are smaller than accompanying increases in N2 densities. The observations support earlier studies suggesting that (1) N densities increase more rapidly than O densities during periods of high solar EUV flux and (2) N densities are larger in the summer hemisphere than in the winter hemisphere. A series of passes in February 1983, late in the lifetime of DE 2, indicated N densities at 200 km altitude were a factor of 2 larger near the southern cusp than near the northern cusp.

  17. Interactions between Rydberg atoms and ultracold polar molecules

    NASA Astrophysics Data System (ADS)

    Jayaseelan, Maitreyi; Haruza, Marek; Bigelow, Nicholas P.

    2015-05-01

    We investigate dipolar interactions arising in a hybrid system containing both ultracold polar molecules and atomic Rydberg states. Ultracold NaCs molecules are produced by photoassociation from laser cooled mixtures of sodium and cesium atoms and detected through resonant multi-photon ionization (REMPI). Rydberg atoms with large dipole moments are excited in the atomic cloud using a multi-photon process and detected via field-ionization. We look for evidence of the interactions in the observed spectra.

  18. Enhanced sensitivity in H photofragment detection by two-color reduced-Doppler ion imaging

    SciTech Connect

    Epshtein, Michael; Portnov, Alexander; Kupfer, Rotem; Rosenwaks, Salman; Bar, Ilana

    2013-11-14

    Two-color reduced-Doppler (TCRD) and one-color velocity map imaging (VMI) were used for probing H atom photofragments resulting from the ∼243.1 nm photodissociation of pyrrole. The velocity components of the H photofragments were probed by employing two counterpropagating beams at close and fixed wavelengths of 243.15 and 243.12 nm in TCRD and a single beam at ∼243.1 nm, scanned across the Doppler profile in VMI. The TCRD imaging enabled probing of the entire velocity distribution in a single pulse, resulting in enhanced ionization efficiency, as well as improved sensitivity and signal-to-noise ratio. These advantages were utilized for studying the pyrrole photodissociation at ∼243.1 and 225 nm, where the latter wavelength provided only a slight increase in the H yield over the self-signal from the probe beams. The TCRD imaging enabled obtaining high quality H{sup +} images, even for the low H photofragment yields formed in the 225 nm photolysis process, and allowed determining the velocity distributions and anisotropy parameters and getting insight into pyrrole photodissociation.

  19. The role of fullerene shell upon stuffed atom polarization potential

    NASA Astrophysics Data System (ADS)

    Amusia, Miron; Chernysheva, Larissa

    2016-05-01

    We have demonstrated that the polarization of the fullerene shell considerably alters the polarization potential of an atom, stuffed inside a fullerene. This essentially affects the electron elastic scattering phases as well as corresponding cross-sections. We illustrate the general trend by concrete examples of electron scattering upon endohedrals that are formed when Ne and Ar atom are stuffed inside fullerene C60. To obtain the presented results, we have suggested a simplified approach that permits to incorporate the effect of fullerenes polarizability into the endohedrals polarization potential. By applying this approach, we obtained numeric results that show strong variations in shape and magnitudes of scattering phases and cross-sections due to effect of fullerene polarization upon the endohedral polarization potential. Using concrete examples we have demonstrated that the elastic scattering of electrons upon endohedrals is an entirely quantum mechanical process, where addition of even a single atom can qualitatively alter the multi-particle cross-section.

  20. VCSEL polarization control for chip-scale atomic clocks.

    SciTech Connect

    Geib, Kent Martin; Peake, Gregory Merwin; Wendt, Joel Robert; Serkland, Darwin Keith; Keeler, Gordon Arthur

    2007-01-01

    Sandia National Laboratories and Mytek, LLC have collaborated to develop a monolithically-integrated vertical-cavity surface-emitting laser (VCSEL) assembly with controllable polarization states suitable for use in chip-scale atomic clocks. During the course of this work, a robust technique to provide polarization control was modeled and demonstrated. The technique uses deeply-etched surface gratings oriented at several different rotational angles to provide VCSEL polarization stability. A rigorous coupled-wave analysis (RCWA) model was used to optimize the design for high polarization selectivity and fabrication tolerance. The new approach to VCSEL polarization control may be useful in a number of defense and commercial applications, including chip-scale atomic clocks and other low-power atomic sensors.

  1. Michigan ultra-cold polarized atomic hydrogen jet target

    NASA Astrophysics Data System (ADS)

    Blinov, B. B.; Gladycheva, S. E.; Kageya, T.; Kantsyrev, D. Yu.; Krisch, A. D.; Luppov, V. G.; Morozov, V. S.; Murray, J. R.; Raymond, R. S.; Borisov, N. S.; Fimushkin, V. V.; Grishin, V. N.; Mysnik, A. I.; Kleppner, D.

    2001-06-01

    To study spin effects in high energy collisions, we are developing an ultra-cold high-density jet target of proton-spin-polarized hydrogen atoms. The target uses a 12 Tesla magnetic field and a 0.3 K separation cell coated with superfluid helium-4 to produce a slow monochromatic electron-spin-polarized atomic hydrogen beam, which is then focused by a superconducting sextupole into the interaction region. In recent tests, we studied a polarized beam of hydrogen atoms focused by the superconducting sextupole into a compression tube detector, which measured the polarized atoms' intensity. The Jet produced, at the detector, a spin-polarized atomic hydrogen beam with a measured intensity of about 2.8.1015 H s-1 and a FWHM area of less than 0.13 cm2. This intensity corresponds to a free jet density of about 1.1012 H cm-3 with a proton polarization of about 50%. When the transition RF unit is installed, we expect a proton polarization higher than 90%. .

  2. Frequency redistribution function for the polarized two-term atom

    SciTech Connect

    Casini, R.; Landi Degl'Innocenti, M.; Manso Sainz, R.; Landolfi, M.

    2014-08-20

    We present a generalized frequency redistribution function for the polarized two-term atom in an arbitrary magnetic field. This result is derived within a new formulation of the quantum problem of coherent scattering of polarized radiation by atoms in the collisionless regime. The general theory, which is based on a diagrammatic treatment of the atom-photon interaction, is still a work in progress. However, the results anticipated here are relevant enough for the study of the magnetism of the solar chromosphere and of interest for astrophysics in general.

  3. Nuclear polarization in heavy atoms and superheavy quasiatoms

    SciTech Connect

    Plunien, G. ); Mueller, B.; Greiner, W. ); Soff, G. )

    1991-06-01

    We consider the contribution of nuclear polarization to the Lamb shift of {ital K}- and {ital L}-shell electrons in heavy atoms and quasiatoms. Our formal approach is based on the concept of effective photon propagators with nuclear-polarization insertions treating effects of nuclear polarization on the same footing as usual QED radiative corrections. We explicitly derive the modification of the photon propagator for various collective nuclear excitations and calculate the corresponding effective self-energy shift perturbatively. The energy shift of the 1{ital s}{sub 1/2} state in {sub 92}{sup 238}U due to virtual excitation of nuclear rotational states is shown to be a considerable correction for atomic high-precision experiments. In contrast to this, nuclear-polarization effects are of minor importance for Lamb-shift studies in {sub 82}{sup 208}Pb.

  4. The effect of electron scattering redistribution on atomic line polarization

    NASA Astrophysics Data System (ADS)

    Supriya, H. D.; Nagendra, K. N.; Sampoorna, M.; Ravindra, B.

    2012-09-01

    The polarization of spectral lines is generated by the scattering of angularly anisotropic incident radiation field on the atoms in the stellar atmosphere. This atomic scattering polarization is modified by frequency non-coherent scattering of line photons on free electrons. With modern spectropolarimeters of high sensitivity, it is possible to detect such changes in the spectral line polarization caused by scattering on electrons. We present new and efficient numerical techniques to solve the problem of line radiative transfer with atomic and electron scattering frequency redistribution in planar media. The evaluation and use of angle-dependent partial frequency redistribution functions (both atomic and electron scattering type) in the transfer equation require a lot of computing effort. In this paper, we apply a decomposition technique to handle this numerically difficult problem. This recently developed technique is applied for the first time to the electron scattering partial redistribution. This decomposition technique allows us to devise fast iterative methods of solving the polarized line transfer equation. An approximate lambda iteration (ALI) method and a method based on Neumann series expansion of the polarized source vector are proposed. We show that these numerical methods can be used to obtain a solution of the problem, when both atomic and electron scattering partial frequency redistribution are considered together. This is in contrast with the classical numerical methods which require a great amount of computing time. We show the importance of electron scattering redistribution in the far wing line polarization, which has practical implications in the analysis of polarized stellar or solar spectra, where non-coherent electron scattering controls the line wing transfer.

  5. Frequency Redistribution of Polarized Light in the Λ-Type Multi-Term Polarized Atom

    NASA Astrophysics Data System (ADS)

    Casini, R.; Manso Sainz, R.

    2016-06-01

    We study the effects of Rayleigh and Raman scattering on the formation of polarized spectral lines in a Λ-type multi-term atom. We fully take into account the partial redistribution of frequency and the presence of atomic polarization in the lower states of the atomic model. Problems that can be modeled with this formalism include, for example, the formation of the Ca ii H–K and IR triplet, the analogous system of Ba ii, and the Lyβ–Hα system of hydrogenic ions.

  6. Role of a fullerene shell upon stuffed atom polarization potential

    NASA Astrophysics Data System (ADS)

    Amusia, M. Ya.; Chernysheva, L. V.

    2016-02-01

    We have demonstrated that the polarization of the fullerene shell considerably alters the polarization potential of an atom, stuffed inside a fullerene. This essentially affects the electron elastic scattering phases as well as corresponding cross sections. We illustrate the general trend by particular examples of electron scattering upon endohedrals Ne@C60 and Ar@C60. To obtain the presented results, we have suggested a simplified approach that permits to incorporate the effect of fullerenes polarizability into the Ne@C60 and Ar@C60 polarization potential. By applying this approach, we obtained numeric results that show strong variations in shape and magnitudes of scattering phases and cross sections due to effect of fullerene polarization upon the endohedral polarization potential.

  7. Magnetism and spin-polarized transport in carbon atomic wires

    NASA Astrophysics Data System (ADS)

    Li, Z. Y.; Sheng, W.; Ning, Z. Y.; Zhang, Z. H.; Yang, Z. Q.; Guo, H.

    2009-09-01

    We report ab initio calculations of magnetic and spin-polarized quantum transport properties of pure and nitrogen-doped carbon atomic wires. For finite-sized wires with even number of carbon atoms, total magnetic moment of 2μB is found. On the other hand, wires with odd number atoms have no net magnetic moment. Doped with one or two nitrogen atom(s), the carbon atomic wires exhibit a spin-density-wave-like state. The magnetic properties can be rationalized through bonding patterns and unpaired states. When the wire is sandwiched between Au electrodes to form a transport junction, perfect spin filtering effect can be induced by slightly straining the wire.

  8. Magnetic-sublevel atomic kinetics modeling for line polarization spectroscopy

    SciTech Connect

    Hakel, P.; Mancini, R. C.

    2004-01-01

    We discuss the mechanism of polarized X-ray line emission in plasmas, its connection to plasma anisotropy, and introduce an atomic kinetics model and code (POLAR) based on the population kinetics of magnetic sublevels. POLAR represents a multi-level, multi-process approach to the problem of polarized spectra in plasmas, and hence it is well suited for plasma applications where cascade effects and alignment transfer can become important. Polarization degrees of X-ray spectral lines computed with POLAR were successfully benchmarked against calculations done with other formalisms, and experimental results obtained at the EBIT facility of Lawrence Livermore National Laboratory. We also investigated the polarization of He-like Si X-ray satellite lines as spectral signatures of anisotropy in the electron distribution function. A comprehensive modeling study was performed taking into account hydrodynamics and electron kinetics. We find that two satellite lines connecting singlet states develop a noticeable polarization while the triplet lines remain unpolarized. These results suggest a scenario where triplet lines could be used as a reference while the singlets could be used as polarized markers of plasma anisotropy.

  9. Atomic and Electronic Structure of Polar Oxide Interfaces

    SciTech Connect

    Gajdardziska-Josifovska, Marija

    2014-01-17

    In this project we developed fundamental understanding of atomic and electronic mechanisms for stabilization of polar oxide interfaces. An integrated experimental and theoretical methodology was used to develop knowledge on this important new class of ionic materials with limited dimensionality, with implications for multiple branches of the basic and applied energy sciences.

  10. Spin-polarized currents generated by magnetic Fe atomic chains.

    PubMed

    Lin, Zheng-Zhe; Chen, Xi

    2014-06-13

    Fe-based devices are widely used in spintronics because of high spin-polarization and magnetism. In this work, freestanding Fe atomic chains, the thinnest wires, were used to generate spin-polarized currents due to the spin-polarized energy bands. By ab initio calculations, the zigzag structure was found to be more stable than the wide-angle zigzag structure and had a higher ratio of spin-up and spin-down currents. By our theoretical prediction, Fe atomic chains have a sufficiently long thermal lifetime only at T ≦̸ 150 K, while C atomic chains are very stable even at T = 1000 K. This means that the spintronic devices based on Fe chains could work only at low temperatures. A system constructed by a short Fe chain sandwiched between two graphene electrodes could be used as a spin-polarized current generator, while a C chain could not be used in this way. The present work may be instructive and meaningful to further practical applications based on recent technical developments on the preparation of metal atomic chains (Proc. Natl. Acad. Sci. USA 107 9055 (2010)). PMID:24849670

  11. ATOMIC BEAM POLARIZATION MEASUREMENT OF THE RHIC POLARIZED H-JET TARGET.

    SciTech Connect

    MAKDISI,Y.; NASS,A.; GRAHAM,D.; KPONOU,A.; MAHLER,G.; MENG,W.; RITTER,J.; ET AL.

    2005-01-28

    The RHIC polarized H-Jet measures the polarization of the RHIC proton beam via elastic scattering off a nuclear polarized atomic hydrogen beam. The atomic beam is produced by a dissociator, a beam forming system and sextupole magnets. Nuclear polarization is achieved by exchanging occupation numbers of hyperfine states using high frequency transitions. The polarization was measured using a modified form of a Breit-Rabi polarimeter including focusing magnets and another set of high frequency transitions. The sampling of a large part of the beam and low noise electronics made it possible to measure the polarization to a high degree of accuracy in a very short time period (1 min). Using this system, we measured no depolarization of the atomic beam due to the RF fields of the bunched proton beam. Time-of-Flight measurements were done using a fast chopper and a QMA at the position of the RHIC interaction point to determine the areal density of the atomic beam seen by the RHIC beam.

  12. Polarized noble-gas atoms: A tool for fundamental physics

    SciTech Connect

    Chupp, T.E.

    1993-05-01

    Polarized noble gas atom samples suitable for a variety of experiments can be produced by spin exchange with laser optically pumped alkali-metal vapors. Most stable and even radioactive isotopes of He, Ne, Kr, Xe and Rn have been polarized, and the field has been paced, in part by laser developments and study of the atomic collision processes. I will focus on two kinds of application: (1) precision measurement of free precession frequencies to probe fundamental concepts such as CP violation, Local Lorentz Invariance and Linearity in Quantum Mechanics; (2) a polarized {sup 3}He target for electron scattering to extract information on the structure of the neutron. The precision measurement techniques take advantage of long coherence times (measured in hours for {sup 3}He and {sup 21}Ne) and large signal to noise ratios to measure frequency shifts with precision 10{sup -7} Hz in one hour. The polarized {sup 3}He target is used to measure asymmetries in deep inelastic electron scattering which are dominated by the neutron since the proton spins are approximately paired in the ground state of the nucleus. The spin dependent structure function of the neutron is an essential probe of the quark-parton structure of the nucleon. All of these investigations combine fundamental and particle physics motivation with atomic physics and precision measurement techniques in a way that spans many subfields of physics.

  13. Nuclear polarization contribution to the Lamb shift in heavy atoms

    SciTech Connect

    Plunien, G.; Mueller, B.; Greiner, W.; Soff, G.

    1989-05-15

    The energy shift of the 1s/sub 1/2/ state in /sub <2//sub 92//sup 38/U due to virtual excitation of nuclear rotational modes is shown to be a considerable correction for atomic high-precision experiments. In contrast to this, nuclear polarization effects are of minor importance for Lamb-shift studies in /sub <2//sub 82//sup 08/Pb.

  14. Polarization enhanced Nuclear Quadrupole Resonance with an atomic magnetometer

    NASA Astrophysics Data System (ADS)

    Malone, Michael W.; Barrall, Geoffrey A.; Espy, Michelle A.; Monti, Mark C.; Alexson, Dimitri A.; Okamitsu, Jeffrey K.

    2016-05-01

    Nuclear Quadrupole Resonance (NQR) has been demonstrated for the detection of 14-N in explosive compounds. Application of a material specific radio-frequency (RF) pulse excites a response typically detected with a wire- wound antenna. NQR is non-contact and material specific, however fields produced by NQR are typically very weak, making demonstration of practical utility challenging. For certain materials, the NQR signal can be increased by transferring polarization from hydrogen nuclei to nitrogen nuclei using external magnetic fields. This polarization enhancement (PE) can enhance the NQR signal by an order of magnitude or more. Atomic magnetometers (AM) have been shown to improve detection sensitivity beyond a conventional antenna by a similar amount. AM sensors are immune to piezo-electric effects that hamper conventional NQR, and can be combined to form a gradiometer for effective RF noise cancellation. In principle, combining polarization enhancement with atomic magnetometer detection should yield improvement in signal-to-noise ratio that is the product of the two methods, 100-fold or more over conventional NQR. However both methods are even more exotic than traditional NQR, and have never been combined due to challenges in operating a large magnetic field and ultra-sensitive magnetic field sensor in proximity. Here we present NQR with and without PE with an atomic magnetometer, demonstrating signal enhancement greater than 20-fold for ammonium nitrate. We also demonstrate PE for PETN using a traditional coil for detection with an enhancement factor of 10. Experimental methods and future applications are discussed.

  15. Properties of Auger electrons following excitation of polarized atoms by polarized electrons

    NASA Astrophysics Data System (ADS)

    Kupliauskienė, A.; Tutlys, V.

    2009-01-01

    In non-relativistic approximation, the most general expression for differential cross sections describing the properties of Auger-electron emission induced in the excitation of polarized atoms by polarized electrons is obtained for the first time. The ways of the application of the general expressions suitable for the specific experimental conditions are outlined by deriving the expressions for the asymmetry parameters and the magnetic dichroism of the angular distribution of the Auger electrons as well as of the angular correlations between the scattered and Auger electrons.

  16. Ultraviolet photodissociation of C2F5I with a small and simple photofragment translational spectrometer.

    PubMed

    Yu, Zijun; Xu, Xiling; Cheng, Min; Yu, Dan; Du, Yikui; Zhu, Qihe

    2009-07-28

    Photodissociation dynamics of C(2)F(5)I near 280 and 304 nm has been investigated on a small and simple time-of-flight photofragment translational spectrometer (PTS). On this new PTS, the photolyzed and ionized fragments, not accelerated by electric field, travel freely for a short flight path (<50 mm) and are detected by microchannel plates. In the spectra of the I(*)((2)P(1/2)) channel at 281.73 and 304.02 nm, vibrational peaks with spacing of approximately 350 cm(-1) are partially resolved, indicating the preferential excitation of CF(2) wag mode (nu(11)=366 cm(-1)) of C(2)F(5) photofragment. The fraction of the available energy disposed into the internal energy is higher than 50% for both I(*) channel and I channel, showing the high excitation of vibration in the C(2)F(5) fragments. The fragment recoil anisotropy parameter beta(I(*)), determined to be 1.70 at 281.73 nm and 1.64 at 304.02 nm, reveals that I(*) atoms are produced predominantly from the parallel (3)Q(0) <-- N transition. The anisotropy parameter beta(I), determined to be 1.25 at 279.71 nm and 0.88 at 304.67 nm, implies that I atoms are produced from two excited states, i.e., direct dissociation via the perpendicular (3)Q(1) <-- N transition, and indirect dissociation via the parallel (3)Q(0) <-- N transition then curve crossing to the (1)Q(1) potential energy surface. Analysis on the recent studies with vibrational state resolution in the photodissociation of alkyl iodides in the A band reveals that the "symmetric bending" mode on alpha-carbon of alkyl iodides is the preferential vibrational excitation mode, which can be explained by the classic impulsive model. PMID:19655883

  17. Magnetic-field-assisted atomic polarization spectroscopy of 4 He

    NASA Astrophysics Data System (ADS)

    Li, Sheng; Wang, Haidong; Wu, Teng; Peng, Xiang; Guo, Hong; Cream Team

    2016-05-01

    Atomic polarization spectroscopy (PS) is a high resolution sub-Doppler atomic spectroscopic technique with free modulation. It is always desirable to obtain a PS signal with zero background as it can provide a more preferable laser frequency stabilization performance. There are many factors that can affect the PS signal background, i.e., the laser power, the laser polarization and the magnetic field. Here, we demonstrate a method for observing and analyzing the effects on the PS signal of 4 He under different magnetic fields. At the beginning, under nearly zero magnetic field, the large asymmetrical PS signal background has been observed and cannot be eliminated by only optically adjusting. Then, we find that the PS signal profile can be changed and controlled by varying the magnetic field with transverse or longitudinal direction and different intensity. The optimized PS signal with symmetrical dispersive profile and zero background is obtained when the magnetic field is chosen and controlled in the transverse direction and more than 20000nT intensity. Similar phenomenon cannot be observed under the longitudinal magnetic field. A theoretical model is also presented, which explains and agrees well with our experimental results.

  18. Resonant quenching of Rydberg atomic states by highly polar molecules

    NASA Astrophysics Data System (ADS)

    Narits, A. A.; Mironchuk, E. S.; Lebedev, V. S.

    2016-06-01

    The results of theoretical studies of the resonant quenching and ion-pair formation processes induced by collisions of Rydberg atoms with highly polar molecules possessing small electron affinities are reported. We elaborate an approach for describing collisional dynamics of both processes and demonstrate the predominant role of resonant quenching channel of reaction for the destruction of Rydberg states by electron-attaching molecules. The approach is based on the solution of the coupled differential equations for the transition amplitudes between the ionic and Rydberg covalent terms of a quasimolecule formed during a collision of particles. It takes into account the possibility of the dipole-bound anion decay in the Coulomb field of the positive ionic core and generalizes previous models of charge-transfer processes involving Rydberg atoms to the cases, when the multistate Landau–Zener approaches become inapplicable. Our calculations for {{Rb}}({nl}) atom perturbed by {{{C}}}2{{{H}}}4{{SO}}3, {{CH}}2{CHCN}, {{CH}}3{{NO}}2, {{CH}}3{CN}, {{{C}}}3{{{H}}}2{{{O}}}3, and {{{C}}}3{{{H}}}4{{{O}}}3 molecules show that the curves representing the dependence of the resonant quenching cross sections on the principal quantum number n are bell-shaped with the positions of maxima being shifted towards lower values of n and the peak values, {σ }{max}({{q})}, several times higher than those for the ion-pair formation, {σ }{max}({{i})}. We obtain a simple power relation between the energy of electron affinity of a molecule and the position of maximum in n-dependence of the resonant quenching cross section. It can be used as an additional means for determining small binding energies of dipole-bound anions from the experimental data on resonant quenching of Rydberg states by highly polar molecules.

  19. Status of the hydrogen and deuterium atomic beam polarized target for NEPTUN experiment

    NASA Astrophysics Data System (ADS)

    Balandikov, N. I.; Ershov, V. P.; Fimushkin, V. V.; Kulikov, M. V.; Pilipenko, Yu. K.; Shutov, V. B.

    1995-09-01

    NEPTUN-NEPTUN-A is a polarized experiment at Accelerating and Storage Complex (UNK, IHEP) with two internal targets. Status of the atomic beam polarized target that is being developed at the Joint Institute for Nuclear Research, Dubna is presented.

  20. Reaction mechanism studies of unsaturated molecules using photofragment translational spectroscopy

    SciTech Connect

    Longfellow, C.A. |

    1996-05-01

    A number of molecules have been studied using the technique of photofragment translational spectroscopy. In Chapter One a brief introduction to the experimental technique is given. In Chapter Two the infrared multiphoton dissociation (IRMPD) of acetic acid is discussed. Carbon dioxide and methane were observed for the first time as products from dissociation under collisionless conditions. Chapter Three relates an IRMPD experiment of hexafluoropropene. The predominant channel produces CFCF{sub 3} or C{sub 2}F{sub 4} and CF{sub 2}, with the heavier species undergoing further dissociation to two CF{sub 2} fragments. In Chapter Four the ultraviolet (UV) dissociation of hexafluoropropene is investigated. Chapter Five explores the IRMPD of octafluoro-1-butene and octafluoro-2-butene.

  1. Photofragment translational spectroscopy of three body dissociations and free radicals

    SciTech Connect

    North, S.W.

    1995-04-01

    This dissertation describes several three-body dissociations and the photodissociation of methyl radicals studied using photofragment translational spectroscopy. The first chapter provides an introduction to three body dissociation, examines current experimental methodology, and includes a discussion on the treatment of photofragment translational spectroscopy data arising from three-body fragmentation. The ultraviolet photodissociation of azomethane into two methyl radicals and nitrogen is discussed in chapter 2. Chapter 3 describes the photodissociation of acetone at 248 nm and 193 nm. At 248 nm the translational energy release from the initial C-C bond cleavage matches the exit barrier height and a comparison with results at 266 nm suggests that is invariant to the available energy. A fraction of the nascent CH{sub 3}CO radicals spontaneously dissociate following rotational averaging. The for the second C-C bond cleavage also matches the exit barrier height. At 193 nm the experimental data can be successfully fit assuming that the dynamics are analogous to those at 248 nm. A simplified model of energy partitioning which adequately describes the experimental results is discussed. Experiments on acetyl halides provide additional evidence to support the proposed acetone dissociation mechanism. A value of 17.0{+-}1.0 kcal/mole for the barrier height, CH{sub 3}CO decomposition has been determined. The photodissociation of methyl radical at 193 nm and 212.8 nm is discussed in the chapter 5. The formation of CH{sub 2} ({sup 1}A{sub l}) and H ({sup 2}S) was the only single photon dissociation pathway observed at both wavelengths.

  2. Effects of atomic hydrogen and deuterium exposure on high polarization GaAs photocathodes

    SciTech Connect

    M. Baylac; P. Adderley; J. Brittian; J. Clark; T. Day; J. Grames; J. Hansknecht; M. Poelker; M. Stutzman; A. T. Wu; A. S. Terekhov

    2005-12-01

    Strained-layer GaAs and strained-superlattice GaAs photocathodes are used at Jefferson Laboratory to create high average current beams of highly spin-polarized electrons. High electron yield, or quantum efficiency (QE), is obtained only when the photocathode surface is atomically clean. For years, exposure to atomic hydrogen or deuterium has been the photocathode cleaning technique employed at Jefferson Laboratory. This work demonstrates that atomic hydrogen cleaning is not necessary when precautions are taken to ensure that clean photocathode material from the vendor is not inadvertently dirtied while samples are prepared for installation inside photoemission guns. Moreover, this work demonstrates that QE and beam polarization can be significantly reduced when clean high-polarization photocathode material is exposed to atomic hydrogen from an rf dissociator-style atomic hydrogen source. Surface analysis provides some insight into the mechanisms that degrade QE and polarization due to atomic hydrogen cleaning.

  3. High-intensity pulsed source of polarized protons with an atomic beam

    SciTech Connect

    Belov, A.S.; Esin, S.K.; Kubalov, S.A.; Kuzik, V.E.; Stepanov, A.A.; Yakushev, V.P.

    1985-10-25

    A source of polarized protons with a beam current up to 2.5 mA in the pulse, a degree of polarization 0.78 +- 0.01, a current pulse length of 120 ..mu..s, and a repetition frequency of 1 Hz is described. This is the first source of polarized protons which makes use of the charge exchange of polarized hydrogen atoms with ions of a deuterium plasma.

  4. Characteristics of Spontaneous Emission of Polarized Atoms in Metal Dielectric Multiple Layer Structures

    NASA Astrophysics Data System (ADS)

    Zhao, Li-Ming; Gu, Ben-Yuan; Zhou, Yun-Song

    2007-11-01

    The spontaneous emission (SE) progress of polarized atoms in a stratified structure of air-dielectric(D0)-metal(M)-dielectric(D1)-air can be controlled effectively by changing the thickness of the D1 layer and rotating the polarized direction of atoms. It is found that the normalized SE rate of atoms located inside the D0 layer crucially depends on the atomic position and the thickness of the D1 layer. When the atom is located near the D0-M interface, the normalized atomic SE rate as a function of the atomic position is abruptly onset for the thin D1 layer. However, with the increasing thickness of the D1 layer, the corresponding curve profile exhibits plateau and stays nearly unchanged. The substantial change of the SE rate stems from the excitation of the surface plasmon polaritons in metal-dielectric interface, and the feature crucially depends on the thickness of D1 layer. If atoms are positioned near the D0-air interface, the substantial variation of the normalized SE rate appears when rotating the polarized direction of atoms. These findings manifest that the atomic SE processes can be flexibly controlled by altering the thickness of the dielectric layer D1 or rotating the orientation of the polarization of atoms.

  5. Anisotropy Modeling of Terahertz Metamaterials: Polarization Dependent Resonance Manipulation by Meta-Atom Cluster

    NASA Astrophysics Data System (ADS)

    Jung, Hyunseung; in, Chihun; Choi, Hyunyong; Lee, Hojin

    2014-06-01

    Recently metamaterials have inspired worldwide researches due to their exotic properties in transmitting, reflecting, absorbing or refracting specific electromagnetic waves. Most metamaterials are known to have anisotropic properties, but existing anisotropy models are applicable only to a single meta-atom and its properties. Here we propose an anisotropy model for asymmetrical meta-atom clusters and their polarization dependency. The proposed anisotropic meta-atom clusters show a unique resonance property in which their frequencies can be altered for parallel polarization, but fixed to a single resonance frequency for perpendicular polarization. The proposed anisotropic metamaterials are expected to pave the way for novel optical systems.

  6. Anisotropy Modeling of Terahertz Metamaterials: Polarization Dependent Resonance Manipulation by Meta-Atom Cluster

    PubMed Central

    Jung, Hyunseung; In, Chihun; Choi, Hyunyong; Lee, Hojin

    2014-01-01

    Recently metamaterials have inspired worldwide researches due to their exotic properties in transmitting, reflecting, absorbing or refracting specific electromagnetic waves. Most metamaterials are known to have anisotropic properties, but existing anisotropy models are applicable only to a single meta-atom and its properties. Here we propose an anisotropy model for asymmetrical meta-atom clusters and their polarization dependency. The proposed anisotropic meta-atom clusters show a unique resonance property in which their frequencies can be altered for parallel polarization, but fixed to a single resonance frequency for perpendicular polarization. The proposed anisotropic metamaterials are expected to pave the way for novel optical systems. PMID:24910144

  7. Measurement of the correlation between electron spin and photon linear polarization in atomic-field bremsstrahlung.

    PubMed

    Tashenov, S; Bäck, T; Barday, R; Cederwall, B; Enders, J; Khaplanov, A; Poltoratska, Yu; Schässburger, K-U; Surzhykov, A

    2011-10-21

    Atomic-field bremsstrahlung has been studied with a longitudinally polarized electron beam. The correlation between the initial orientation of the electron spin and the angle of photon polarization has been measured at the photon high energy tip region. In the time reversal this corresponds to a so-far unobserved phenomenon of production of longitudinally polarized electrons by photoionization of unpolarized atoms with linearly polarized photons. The results confirm the fully relativistic calculations for radiative recombination and suggest a new method for electron beam polarimetry. PMID:22107514

  8. Progress on producing polarized negative hydrogen ions by the ETHZ polarized ion source using the atomic beam method

    NASA Astrophysics Data System (ADS)

    Schmelzbach, P. A.; Grüebler, W.

    1983-03-01

    The progress on the ETHZ polarized negative hydrogen ion source, based on the atomic beam method, is described. Particular improvements have been made in the double charge exchange from positive to negative hydrogen ions. At present the source produces over 100 μA H+ ions, which yields 5-6 μA polarized negative hydrogen ions. These ions have been accelerated, in a EN tandem accelerator. A record current of 2-3 μA of polarized deuterons with 89% polarization could be focused through a 3 mm diameter collimator on a target. Further improvements incorporating presently available techniques are discussed. It is shown that 50-100 μA of polarized H- and D- ions can be produced with this type of source.

  9. Decomposing the First Absorption Band of OCS Using Photofragment Excitation Spectroscopy.

    PubMed

    Toulson, Benjamin W; Murray, Craig

    2016-09-01

    Photofragment excitation spectra of carbonyl sulfide (OCS) have been recorded from 212-260 nm by state-selectively probing either electronically excited S((1)D) or ground state S((3)P) photolysis products via 2 + 1 resonance-enhanced multiphoton ionization. Probing the major S((1)D) product results in a broad, unstructured action spectrum that reproduces the overall shape of the first absorption band. In contrast, spectra obtained probing S((3)P) products display prominent resonances superimposed on a broad continuum; the resonances correspond to the diffuse vibrational structure observed in the conventional absorption spectrum. The vibrational structure is assigned to four progressions, each dominated by the C-S stretch, ν1, following direct excitation to quasi-bound singlet and triplet states. The S((3)PJ) products are formed with a near-statistical population distribution over the J = 2, 1, and 0 spin-orbit levels across the wavelength range investigated. Although a minor contributor to the S atom yield near the peak of the absorption cross section, the relative yield of S((3)P) increases significantly at longer wavelengths. The experimental measurements validate recent theoretical work characterizing the electronic states responsible for the first absorption band by Schmidt and co-workers. PMID:27552402

  10. Photofragment image analysis using the Onion-Peeling Algorithm

    NASA Astrophysics Data System (ADS)

    Manzhos, Sergei; Loock, Hans-Peter

    2003-07-01

    With the growing popularity of the velocity map imaging technique, a need for the analysis of photoion and photoelectron images arose. Here, a computer program is presented that allows for the analysis of cylindrically symmetric images. It permits the inversion of the projection of the 3D charged particle distribution using the Onion Peeling Algorithm. Further analysis includes the determination of radial and angular distributions, from which velocity distributions and spatial anisotropy parameters are obtained. Identification and quantification of the different photolysis channels is therefore straightforward. In addition, the program features geometry correction, centering, and multi-Gaussian fitting routines, as well as a user-friendly graphical interface and the possibility of generating synthetic images using either the fitted or user-defined parameters. Program summaryTitle of program: Glass Onion Catalogue identifier: ADRY Program Summary URL:http://cpc.cs.qub.ac.uk/summaries/ADRY Program obtainable from: CPC Program Library, Queen's University of Belfast, N. Ireland Licensing provisions: none Computer: IBM PC Operating system under which the program has been tested: Windows 98, Windows 2000, Windows NT Programming language used: Delphi 4.0 Memory required to execute with typical data: 18 Mwords No. of bits in a word: 32 No. of bytes in distributed program, including test data, etc.: 9 911 434 Distribution format: zip file Keywords: Photofragment image, onion peeling, anisotropy parameters Nature of physical problem: Information about velocity and angular distributions of photofragments is the basis on which the analysis of the photolysis process resides. Reconstructing the three-dimensional distribution from the photofragment image is the first step, further processing involving angular and radial integration of the inverted image to obtain velocity and angular distributions. Provisions have to be made to correct for slight distortions of the image, and to

  11. Two-photon ionization of atomic hydrogen with elliptically polarized light

    NASA Technical Reports Server (NTRS)

    Kassaee, A.; Rustgi, M. L.; Long, S. A. T.

    1988-01-01

    The theory of two-photon ionization of a hydrogenic state in the nonrelativistic dipole approximation is generalized for elliptically polarized light. An application to the metastable 2S state of atomic hydrogen is made. Significant differences in the angular distribution of the outgoing electrons are found depending upon the polarization of the photons. It is claimed that two-photon ionization employing elliptically polarized photons from lasers may provide an additional test for the theories of multiphoton ionization.

  12. (2+1) laser-induced fluorescence of spin-polarized hydrogen atoms.

    PubMed

    Bougas, Lykourgos; Sofikitis, Dimitris; Everest, Michael A; Alexander, Andrew J; Rakitzis, T Peter

    2010-11-01

    We report the measurement of the spin polarization of hydrogen (SPH) atoms by (2+1) laser-induced fluorescence, produced via the photodissociation of thermal HBr molecules with circularly polarized 193 nm light. This scheme, which involves two-photon laser excitation at 205 nm and fluorescence at 656 nm, offers an experimentally simpler polarization-detection method than the previously reported vacuum ultraviolet detection scheme, allowing the detection of SPH atoms to be performed more straightforwardly, from the photodissociation of a wide range of molecules and from a variety of collision experiments. PMID:21054033

  13. Systematically investigating the polarization gradient cooling in an optical molasses of ultracold cesium atoms

    NASA Astrophysics Data System (ADS)

    Ji, Zhong-Hua; Yuan, Jin-Peng; Zhao, Yan-Ting; Chang, Xue-Fang; Xiao, Lian-Tuan; Jia, Suo-Tang

    2014-11-01

    We systematically investigate the polarization gradient cooling (PGC) process in an optical molasses of ultracold cesium atoms. The SR mode for changing the cooling laser, which means that the cooling laser frequency is stepped to the setting value while its intensity is ramped, is found to be the best for the PGC, compared with other modes studied. We verify that the heating effect of the cold atoms, which appears when the cooling laser intensity is lower than the saturation intensity, arises from insufficient polarization gradient cooling. Finally, an exponential decay function with a statistical explanation is introduced to explain the dependence of the cold atom temperature on the PGC interaction time.

  14. Production of excited atomic hydrogen and deuterium from H2 and D2photodissociation

    SciTech Connect

    Bozek, J.D.; Furst, J.E.; Gay, T.J.; Gould, H.; Kilcoyne, A.L.D.; Machacek, J.R.; Martin, F.; McLaughlin, K.W.; Sanz-Vicario, J.L.

    2006-09-17

    We have measured the production of both Ly alpha and H alphafluorescence from atomic H and D for the photodissociation of H2 and D2by linearly polarized photons with energies between 24 and 60 eV. In thisenergy range, excited photofragments result primarily from the productionof doubly excited molecular species which promptly autoionize ordissociate into two neutrals. Our data are compared with ab initiocalculations of the dissociation process, in which both doubly excitedstate production and prompt ionization (nonresonant) channels areconsidered. Agreement between our experimental data and that of earlierwork, and with our theoretical calculations, is qualitative atbest.

  15. Atomic-scale compensation phenomena at polar interfaces

    SciTech Connect

    Chisholm, Matthew F; Luo, Weidong; Oxley, Mark P; Pantelides, Sokrates T; Lee, Ho Nyung

    2010-01-01

    The interfacial screening charge that arises to compensate electric fields of dielectric or ferroelectric thin films is now recognized as the most important factor in determining the capacitance or polarization of ultrathin ferroelectrics. Here we investigate using aberration-corrected electron microscopy and density-functional theory to show how interfaces cope with the need to terminate ferroelectric polarization. In one case, we show evidence for ionic screening, which has been predicted by theory but never observed. For a ferroelectric film on an insulating substrate, we found that compensation can be mediated by an interfacial charge generated, for example, by oxygen vacancies.

  16. Understanding atomic disorder in polar and magnetic oxides

    NASA Astrophysics Data System (ADS)

    Shoemaker, Daniel P.

    The functional properties of materials rely upon the composition, coordination, and connectivity of their constituent atoms. Understanding the atomic structure of condensed materials permits an understanding of how that structure influences macroscopic properties. The field of crystallography seeks to define the repeating lattice of periodic materials using a unit cell model with the minimum number of specified atomic positions. For magnetic and electronic materials, the arrangement of atoms and dipoles are often both ordered over long ranges and amenable to a traditional crystallographic description. However, interesting phenomena emerge when materials experience disorder due to chemical substitution, phase competition, nanostructuring, interfaces, or valence disproportionation. In those cases, the long-range symmetry of the material is interrupted and traditional crystallographic methods struggle to incorporate disorder into the unit cell model. I will discuss how disorder can be identified and quantified in functional materials. Each study includes examination of the real-space pair distribution function (PDF), which provides a weighted histogram of all atom-atom distances in a sample. Models are created by simultaneous fits to the Bragg profile and the PDF, thereby constraining the atomic positions by reciprocal- and real-space scattering descriptions. The reverse Monte Carlo method drives stochastic fits to scattering data using tens of thousands of atoms. Once simulation is complete, crystallographic metrics can be extracted from the supercell in real space. This approach is discussed in the case of site mixing and valence disproportionation in the Jahn-Teller active spinel CuMn2O4, local Jahn-Teller distortions of CuO4 tetrahedra in the solid solution Mg 1-xCuxCr 2O4, nanoscale phase co-existence at the metal-insulator transition in VO2, and static displacements and lone-pair activity in the pyrochlores Bi2Ti2O6O' and Bi 2Ru2O6O'.

  17. Production of a fully spin-polarized ensemble of positronium atoms.

    PubMed

    Cassidy, D B; Meligne, V E; Mills, A P

    2010-04-30

    Long-lived |m|=1 positronium (Ps) atoms are produced in vacuum when high density bursts of positrons with net polarization p{0} are implanted into a porous silica film in a 2.3 T magnetic field. We observe a decrease in the |m|=1 population as the density of the incident positron beam is increased due to quenching interactions between oppositely polarized Ps atoms within the target. Saturation of this density dependent quenching indicates that the initial positron spin polarization p{0}=28+/-1%, and demonstrates the long term (10{2} s) survival of positron polarization in a Surko-type buffer gas trap. We conclude that, at high Ps densities, the minority spin component is essentially eliminated and the remaining Ps is almost entirely (approximately 96%) polarized, as required for the formation of a Ps Bose-Einstein condensate. PMID:20482106

  18. Electron spin polarization in strong-field ionization of xenon atoms

    NASA Astrophysics Data System (ADS)

    Hartung, Alexander; Morales, Felipe; Kunitski, Maksim; Henrichs, Kevin; Laucke, Alina; Richter, Martin; Jahnke, Till; Kalinin, Anton; Schöffler, Markus; Schmidt, Lothar Ph. H.; Ivanov, Misha; Smirnova, Olga; Dörner, Reinhard

    2016-08-01

    As a fundamental property of the electron, the spin plays a decisive role in the electronic structure of matter, from solids to molecules and atoms, for example, by causing magnetism. Yet, despite its importance, the spin dynamics of the electrons released during the interaction of atoms with strong ultrashort laser pulses has remained experimentally unexplored. Here, we report the experimental detection of electron spin polarization by the strong-field ionization of xenon atoms and support our results with theoretical analysis. We found up to 30% spin polarization changing its sign with electron energy. This work opens the new dimension of spin to strong-field physics. It paves the way to the production of sub-femtosecond spin-polarized electron pulses with applications ranging from probing the magnetic properties of matter at ultrafast timescales to testing chiral molecular systems with sub-femtosecond temporal and sub-ångström spatial resolutions.

  19. State-insensitive trapping of Rb atoms: Linearly versus circularly polarized light

    NASA Astrophysics Data System (ADS)

    Arora, Bindiya; Sahoo, B. K.

    2012-09-01

    We study the cancellation of differential ac Stark shifts in the 5s and 5p states of the rubidium atom using the linearly and circularly polarized lights by calculating their dynamic polarizabilities. Matrix elements were calculated using a relativistic coupled-cluster method at the single and double excitations and at the important valence triple excitation approximation including all possible nonlinear correlation terms. Some of the important matrix elements were further optimized using the experimental results available for the lifetimes and static polarizabilities of atomic states. “Magic wavelengths” are determined from the differential Stark shifts and results for the linearly polarized light are compared with the previously available results. The possible scope of facilitating state-insensitive optical trapping schemes using the magic wavelengths for circularly polarized light is discussed. Using the optimized matrix elements, the lifetimes of the 4d and 6s states of this atom are ameliorated.

  20. Electron elastic scattering off A @C60 : The role of atomic polarization under confinement

    NASA Astrophysics Data System (ADS)

    Dolmatov, V. K.; Amusia, M. Ya.; Chernysheva, L. V.

    2015-10-01

    The present paper explores possible features of electron elastic scattering off endohedral fullerenes A @C60 . It focuses on how dynamical polarization of the encapsulated atom A by an incident electron might alter scattering off A @C60 compared to the static-atom-A case, as well as how the C60 confinement modifies the impact of atomic polarization on electron scattering compared to the free-atom case. The aim is to provide researchers with a "relative frame of reference" for understanding which part of the scattering processes could be due to electron scattering off the encapsulated atom and which could be due to scattering off the C60 cage. To meet the goal, the C60 cage is modeled by an attractive spherical potential of a certain inner radius, thickness, and depth which is a model used frequently in a great variety of fullerene studies to date. Then, the Dyson equation for the self-energy part of the Green's function of an incident electron moving in the combined field of an encapsulated atom A and C60 is solved in order to account for the impact of dynamical polarization of the encaged atom upon e +A @C60 scattering. The Ba@C60 endohedral is chosen as the case study. The impact is found to be significant, and its utterly different role compared to that in e +Ba scattering is unraveled.

  1. Two-electron exchange interaction between polar molecules and atomic ions — Asymptotic approach

    NASA Astrophysics Data System (ADS)

    Karbovanets, Oleksandr M.; Karbovanets, Myroslav I.; Khoma, Mykhaylo V.; Lazur, Volodymyr Yu.

    2015-05-01

    We have described the asymptotic approach for calculation of the two-electron exchange interaction between atomic ion and polar molecule responsible for direct double electron transfer processes. The closed analytic expression for matrix element of exchange interaction has been obtained in the framework of the semiclassical version of the asymptotic theory and point-dipole approximation for description of the polar molecule. Contribution to the Topical Issue "Elementary Processes with Atoms and Molecules in Isolated and Aggregated States", edited by Friedrich Aumayr, Bratislav Marinkovic, Štefan Matejčik, John Tanis and Kurt H. Becker.

  2. Nonadiabatic coupling in cold collisions of spin-polarized metastable hydrogen atoms

    SciTech Connect

    Forrey, Robert C.; Dalgarno, Alex; Vanne, Yulian V.; Saenz, Alejandro; Froelich, Piotr

    2007-11-15

    Previous calculations of low-temperature cross sections for collisions between spin-polarized metastable hydrogen atoms are improved to include nonadiabatic radial and angular coupling at large interatomic separations. The electrostatic dipole-quadrupole interaction produces nonadiabatic radial coupling between (2s,2p) and (2p,2p) states, while the Coriolis interaction produces nonadiabatic angular coupling. Both of these long-range contributions are handled in a space-fixed atomic gauge that is particularly convenient for a spin-polarized system. The improved theoretical results are compared with an existing experiment.

  3. Polarized Atomic Hydrogen Beam Tests in the Michigan Ultra-Cold Jet Target

    NASA Astrophysics Data System (ADS)

    Kageya, T.; Blinov, B. B.; Denbow, J. M.; Kandes, M. C.; Krisch, A. D.; Kulkarni, D. A.; Lehman, M. A.; Luppov, V. G.; Morozov, V. S.; Murray, J. R.; Peters, C. C.; Raymond, R. S.; Ross, M. R.; Yonehara, K.; Borisov, N. S.; Fimushkin, V. V.; Kleppner, D.; Grishin, V. N.; Mysnik, A. L.

    2001-04-01

    To study spin effects in high energy collisions, we are developing an ultra-cold high-density jet target of proton-spin-polarized hydrogen atoms (Michigan Jet Target). The target uses a 12 Tesla magnetic field and a 0.3 K separation cell coated with superfluid helium-4 to produce a slow monochromatic electron-spin-polarized atomic hydrogen beam; an rf transition unit then converts this into a proton-spin-polarized beam, which is focused by a superconducting sextupole into the interaction region. The Jet produced, at the detector, a spin-polarized atomic hydrogen beam with a measured intensity of about 1.7 10^15 H s-1 and a FWHM area of less than 0.13 cm^2. This intensity corresponds to a free jet density of about 1.3 10^12 H cm-3 with a proton polarization of about 50%. When the transition RF unit is installed, we expect a proton polarization higher than 90%.

  4. Optical Polarization From Aligned Atoms As A Diagnostic Of Interstellar And Circumstellar Magnetic Fields

    NASA Astrophysics Data System (ADS)

    Yan, H.; Lazarian, A.

    2005-12-01

    Population among sublevels of the ground state of an atom is affected by radiative transitions induced by anisotropic radiation flux. Such aligned atoms precess in the external magnetic field and this affects properties of polarized radiation arising from both scattering and absorption by atoms. As the result the degree of light polarization depends on the direction of the magnetic field. This provides a perspective tool for studies of astrophysical magnetic fields using optical and UV polarimetry. We discuss the process of alignment that can be used to study magnetic fields in interplanetary medium, interstellar medium, circumstellar regions and quasars. To exemplify what atomic alignment can provide to the observers we consider synthetic data obtained with MHD simulations of comet wake.

  5. A polarized internal sup 3 He target using optical pumping of metastable atoms

    SciTech Connect

    McKeown, R.D.; Milner, R.G.; Woodward, C.E. )

    1989-05-05

    The design of a polarized internal {sup 3}He target for use in storage rings based on optical pumping of metastables is discussed. The target employs an infrared laser to polarize {sup 3}He atoms in a pyrex cell which is connected by a capillary to a windowless cell through which the stored beam passes. Using this technique it should be possible construct targets of 50% polarized {sup 3}He targets of thickness 10{sup 16} cm{sup {minus}2}. Small holding fields ({similar to}10 gauss) and resistance to beam-induced depolarization are desirable features of this target in a storage ring environment.

  6. Shot Noise as a Probe of Spin-Polarized Transport through Single Atoms

    NASA Astrophysics Data System (ADS)

    Burtzlaff, Andreas; Weismann, Alexander; Brandbyge, Mads; Berndt, Richard

    2015-01-01

    Single atoms on Au(111) surfaces have been contacted with the Au tip of a low temperature scanning tunneling microscope. The shot noise of the current through these contacts has been measured up to frequencies of 120 kHz and Fano factors have been determined to characterize the transport channels. The noise at Fe and Co atoms, the latter displaying a Kondo effect, indicates spin-polarized transport through a single channel. Transport calculations reproduce this observation.

  7. Gigahertz Dielectric Polarization of Substitutional Single Niobium Atoms in Defective Graphitic Layers.

    PubMed

    Zhang, Xuefeng; Guo, Junjie; Guan, Pengfei; Qin, Gaowu; Pennycook, Stephen J

    2015-10-01

    We synthesize two Nb/C composites with an order of magnitude difference in the density of single niobium atoms substituted into defective graphitic layers. The concentration and sites of single Nb atoms are identified using aberration-corrected scanning transmission electron microscopy and density functional theory. Comparing the experimental complex permittivity spectra reveals that a representative dielectric resonance at ∼16  GHz originates from the intrinsic polarization of single Nb atom sites, which is confirmed by theoretical simulations. The single-atom dielectric resonance represents the physical limit of the electromagnetic response of condensed matter, and thus might open up a new avenue for designing electromagnetic wave absorption materials. Single-atom resonance also has important implications in understanding the correlation between the macroscopic dielectric behaviors and the atomic-scale structural origin. PMID:26551823

  8. Giant molecules composed of polar molecules and atoms in mixed dimensions

    NASA Astrophysics Data System (ADS)

    Qi, Ran; Tan, Shina

    2014-05-01

    Two or three polar molecules, confined to one or two dimensions, can form stable bound states with a single atom living in three dimensions, if the molecule and the atom can interact resonantly such that their mixed dimensional scattering length is large. We call these bound states ``giant molecules'' since it's a molecule composed of smaller molecules and atoms. We study their properties using techniques including exact numerical solution, exact qunatum diffusion Monte Carlo (QMC), Born-Oppenheimer approximation (BOA), and semiclassical approximation. These bound states have a hierarchical structure reminiscent of the celestial systems.

  9. Polarized Atomic Hydrogen Beam Tests in the Mark-II Ultra-Cold Jet Target.

    NASA Astrophysics Data System (ADS)

    Luppov, V. G.; Blinov, B. B.; Gladycheva, S. E.; Kageya, T.; Kantsyrev, D. Yu.; Krisch, A. D.; Murray, J. R.; Neumann, J. J.; Raymond, R. S.; Borisov, N. S.; Kleppner, D.; Davidenko, A. M.; Grishin, V. N.

    2000-04-01

    To study spin effects in high energy collisions, we are developing an ultra-cold high-density jet target of proton-spin-polarized hydrogen atoms (Mark-II). The target uses a 12 Tesla magnetic field and a 0.3 K separation cell coated with superfluid helium-4 to produce a slow monochromatic electron-spin-polarized atomic hydrogen beam; an rf transition unit then converts this into a proton-spin-polarized beam, which is focused by a superconducting sextupole into the interaction region. Recently, the Jet produced a measured electron-spin-polarized atomic hydrogen beam of about 10^15 H s-1 into a 0.3 cm^2 area at the detector. This intensity corresponds to the free jet density of about 10^11 H cm-3 with a proton polarization of about 50%. So far, the intensity is limited by the high insulation vacuum pressure due to the evaporation of the separation cell's helium film. The beam's angular and radial distributions were measured. A test of a new superfluid-^4He-coated parabolic mirror, attached to the separation cell, appeared to increase the beam intensity by a factor of about 3, as expected.

  10. Photodissociation dynamics of the methyl perthiyl radical at 248 and 193 nm using fast-beam photofragment translational spectroscopy

    NASA Astrophysics Data System (ADS)

    Harrison, Aaron W.; Ryazanov, Mikhail; Sullivan, Erin N.; Neumark, Daniel M.

    2016-07-01

    The photodissociation dynamics of the methyl perthiyl radical (CH3SS) have been investigated using fast-beam coincidence translational spectroscopy. Methyl perthiyl radicals were produced by photodetachment of the CH3SS- anion followed by photodissociation at 248 nm (5.0 eV) and 193 nm (6.4 eV). Photofragment mass distributions and translational energy distributions were measured at each dissociation wavelength. Experimental results show S atom loss as the dominant (96%) dissociation channel at 248 nm with a near parallel, anisotropic angular distribution and translational energy peaking near the maximal energy available to ground state CH3S and S fragments, indicating that the dissociation occurs along a repulsive excited state. At 193 nm, S atom loss remains the major fragmentation channel, although S2 loss becomes more competitive and constitutes 32% of the fragmentation. The translational energy distributions for both channels are very broad at this wavelength, suggesting the formation of the S2 and S atom products in several excited electronic states.

  11. Eigenmode expansion of the polarization for a spherical sample of two-level atoms

    NASA Astrophysics Data System (ADS)

    Friedberg, Richard; Manassah, Jamal T.

    2009-12-01

    We derive pseudo-orthogonality relations for both the magnetic and electric eigenmodes of a system of two-level atoms in a sphere configuration. We verify numerically that an arbitrary vector field can be reconstructed to a great accuracy from these eigenmode expansions. We apply this eigenmode analysis to explore superradiance from a sphere with initially uniform polarization.

  12. Vacuum-polarization contribution to the hyperfine-structure splitting of hydrogenlike atoms

    SciTech Connect

    Schneider, S.M.; Greiner, W. ); Soff, G. )

    1994-07-01

    A calculation of the vacuum-polarization contribution to the hyperfine splitting for hydrogenlike atoms is presented. The extended nuclear charge distribution is taken into account. For the experimentally interesting case [sup 209]Bi[sup 82+] we predict a [Delta][lambda]=[minus]1.6 nm shift for the transition wavelength of the ground-state hyperfine splitting.

  13. Spectroscopic evidence for spin-polarized silicon atoms on Si(553)-Au

    SciTech Connect

    Snijders, Paul C; Johnson, P.S.; Guisinger, Nathan; Erwin, S. C.; Himpsel, F.J.

    2012-01-01

    The stepped Si(553)-Au surface undergoes a $1\\times3$ reconstruction at low temperature which has recently been interpreted theoretically as the $\\times3$ ordering of spin-polarized silicon atoms along a step edge in each surface unit cell. This predicted magnetic ground state has a clear spectroscopic signature---a silicon step-edge state at $0.5$ eV above the Fermi level---that arises from strong exchange splitting and hence would not occur without spin polarization. Here we report spatially resolved scanning tunneling spectroscopy data for Si(553)-Au that reveal key differences in the unoccupied step-edge density of states between room temperature and $40$ K. At low temperature we find an unoccupied state at 0.55 eV above every third step-edge silicon atom, in excellent agreement with the spin-polarized ground state predicted theoretically.

  14. Photoelectron angular distributions in bichromatic atomic ionization induced by circularly polarized VUV femtosecond pulses

    NASA Astrophysics Data System (ADS)

    Douguet, Nicolas; Grum-Grzhimailo, Alexei N.; Gryzlova, Elena V.; Staroselskaya, Ekaterina I.; Venzke, Joel; Bartschat, Klaus

    2016-03-01

    We investigate two-pathway interferences between nonresonant one-photon and resonant two-photon ionization of atomic hydrogen. In particular, we analyze in detail the photoionization mediated by the fundamental frequency and the second harmonic of a femtosecond VUV pulse when the fundamental is tuned near an intermediate atomic state. Following our recent study [Phys. Rev. A 91, 063418 (2015), 10.1103/PhysRevA.91.063418] of such effects with linearly polarized light, we analyze a similar situation with circularly polarized radiation. As a consequence of the richer structure in circularly polarized light, characterized by its right-handed or left-handed helicity, we present and discuss various important features associated with the photoelectron angular distribution.

  15. Switching surface polarization of atomic force microscopy probe utilizing photoisomerization of photochromic molecules

    SciTech Connect

    Aburaya, Yoshihiro; Nomura, Hikaru; Kageshima, Masami; Naitoh, Yoshitaka; Li, Yan Jun; Sugawara, Yasuhiro

    2011-03-15

    An attempt to develop an atomic force microscopy (AFM) probe with optically switchable polarization is described. Modification with a single molecular layer of photochromic molecules was attempted onto a Si substrate that is a prototype for a probe surface. Polarization switching caused by alternate irradiation of UV and visible lights were detected using the electrostatic force?>spectroscopy (EFS) technique. Si substrates modified with spiropyran and azobenzene exhibited reversible polarization switching that caused changes in CPD of about 100 and 50 mV, respectively. Modification with spiropyran was also attempted onto a Si probe and resulted in a CPD change of about 100 mV. It was confirmed that modification of an AFM probe or substrate with a single molecular layer of photochromic molecules can generate surface polarization switching of a mechanically detectable level.

  16. Phase-space structures and ionization dynamics of the hydrogen atom in elliptically polarized microwaves

    NASA Astrophysics Data System (ADS)

    Shchekinova, E.; Chandre, C.; Uzer, T.

    2006-10-01

    The multiphoton ionization of hydrogen atoms in a strong elliptically polarized microwave field exhibits complex features that are not observed for ionization in circular and linear polarized fields. Experimental data reveal high sensitivity of ionization dynamics to the small changes of the field polarization. The multidimensional nature of the problem makes widely used diagnostics of dynamics, such as Poincaré surfaces of section, impractical. We analyze the phase-space dynamics using the finite time stability analysis rendered by the fast Lyapunov indicators technique. The concept of zero-velocity surface is used to initialize the calculations and visualize the dynamics. Our analysis provides stability maps calculated for the initial energy at the maximum and below the saddle of the zero-velocity surface. We estimate qualitatively the dependence of ionization thresholds on the parameters of the applied field, such as polarization and scaled amplitude.

  17. Nonlinear polarization response of a gaseous medium in the regime of atom stabilization in a strong radiation field

    SciTech Connect

    Volkova, E. A.; Popov, A. M. Tikhonova, O. V.

    2013-03-15

    The nonlinear polarization response of a quantum system modeling a silver atom in the field of high-intensity radiation in the IR and UV spectral ranges has been studied by direct numerical integration of a nonstationary Schroedinger equation. The domains of applicability of perturbation theory and polarization expansion in powers of the field intensity are determined. The contribution of excited atoms and electrons in a continuum to the atomic polarization response at the field frequency, which arises due to the radiation-induced excitation and photoionization processes, is analyzed. Features of the nonlinear response to an external field under conditions of atom stabilization are considered.

  18. Telecom-Wavelength Atomic Quantum Memory in Optical Fiber for Heralded Polarization Qubits

    NASA Astrophysics Data System (ADS)

    Jin, Jeongwan; Saglamyurek, Erhan; Puigibert, Marcel. lí Grimau; Verma, Varun; Marsili, Francesco; Nam, Sae Woo; Oblak, Daniel; Tittel, Wolfgang

    2015-10-01

    Polarization-encoded photons at telecommunication wavelengths provide a compelling platform for practical realizations of photonic quantum information technologies due to the ease of performing single qubit manipulations, the availability of polarization-entangled photon-pair sources, and the possibility of leveraging existing fiber-optic links for distributing qubits over long distances. An optical quantum memory compatible with this platform could serve as a building block for these technologies. Here we present the first experimental demonstration of an atomic quantum memory that directly allows for reversible mapping of quantum states encoded in the polarization degree of freedom of a telecom-wavelength photon. We show that heralded polarization qubits at a telecom wavelength are stored and retrieved with near-unity fidelity by implementing the atomic frequency comb protocol in an ensemble of erbium atoms doped into an optical fiber. Despite remaining limitations in our proof-of-principle demonstration such as small storage efficiency and storage time, our broadband light-matter interface reveals the potential for use in future quantum information processing.

  19. Telecom-Wavelength Atomic Quantum Memory in Optical Fiber for Heralded Polarization Qubits.

    PubMed

    Jin, Jeongwan; Saglamyurek, Erhan; Puigibert, Marcel lí Grimau; Verma, Varun; Marsili, Francesco; Nam, Sae Woo; Oblak, Daniel; Tittel, Wolfgang

    2015-10-01

    Polarization-encoded photons at telecommunication wavelengths provide a compelling platform for practical realizations of photonic quantum information technologies due to the ease of performing single qubit manipulations, the availability of polarization-entangled photon-pair sources, and the possibility of leveraging existing fiber-optic links for distributing qubits over long distances. An optical quantum memory compatible with this platform could serve as a building block for these technologies. Here we present the first experimental demonstration of an atomic quantum memory that directly allows for reversible mapping of quantum states encoded in the polarization degree of freedom of a telecom-wavelength photon. We show that heralded polarization qubits at a telecom wavelength are stored and retrieved with near-unity fidelity by implementing the atomic frequency comb protocol in an ensemble of erbium atoms doped into an optical fiber. Despite remaining limitations in our proof-of-principle demonstration such as small storage efficiency and storage time, our broadband light-matter interface reveals the potential for use in future quantum information processing. PMID:26551798

  20. Atomic mechanism of polarization-controlled surface reconstruction in ferroelectric thin films

    PubMed Central

    Gao, Peng; Liu, Heng-Jui; Huang, Yen-Lin; Chu, Ying-Hao; Ishikawa, Ryo; Feng, Bin; Jiang, Ying; Shibata, Naoya; Wang, En-Ge; Ikuhara, Yuichi

    2016-01-01

    At the ferroelectric surface, the broken translational symmetry induced bound charge should significantly alter the local atomic configurations. Experimentally revealing the atomic structure of ferroelectric surface, however, is very challenging due to the strong spatial variety between nano-sized domains, and strong interactions between the polarization and other structural parameters. Here, we study surface structures of Pb(Zr0.2Ti0.8)O3 thin film by using the annular bright-field imaging. We find that six atomic layers with suppressed polarization and a charged 180° domain wall are at negatively poled surfaces, no reconstruction exists at positively poled surfaces, and seven atomic layers with suppressed polarization and a charged 90° domain wall exist at nominally neutral surfaces in ferroelastic domains. Our results provide critical insights into engineering ferroelectric thin films, fine grain ceramics and surface chemistry devices. The state-of-the-art methodology demonstrated here can greatly advance our understanding of surface science for oxides. PMID:27090766

  1. Atomic mechanism of polarization-controlled surface reconstruction in ferroelectric thin films.

    PubMed

    Gao, Peng; Liu, Heng-Jui; Huang, Yen-Lin; Chu, Ying-Hao; Ishikawa, Ryo; Feng, Bin; Jiang, Ying; Shibata, Naoya; Wang, En-Ge; Ikuhara, Yuichi

    2016-01-01

    At the ferroelectric surface, the broken translational symmetry induced bound charge should significantly alter the local atomic configurations. Experimentally revealing the atomic structure of ferroelectric surface, however, is very challenging due to the strong spatial variety between nano-sized domains, and strong interactions between the polarization and other structural parameters. Here, we study surface structures of Pb(Zr0.2Ti0.8)O3 thin film by using the annular bright-field imaging. We find that six atomic layers with suppressed polarization and a charged 180° domain wall are at negatively poled surfaces, no reconstruction exists at positively poled surfaces, and seven atomic layers with suppressed polarization and a charged 90° domain wall exist at nominally neutral surfaces in ferroelastic domains. Our results provide critical insights into engineering ferroelectric thin films, fine grain ceramics and surface chemistry devices. The state-of-the-art methodology demonstrated here can greatly advance our understanding of surface science for oxides. PMID:27090766

  2. Moøller polarimetry with polarized atomic hydrogen at MESA

    SciTech Connect

    Bartolomé, P. Aguar; Aulenbacher, K.; Tyukin, V.

    2013-11-07

    A new generation of parity violation (PV) electron scattering experiments are planned to be carried out at the Institut für Kernphysik in Mainz. These experiments will be performed at low energies of 100-200 MeV using the new accelerator MESA (Mainz Energy recovering Superconducting Accelerator). One of the main challenges of such experiments is to achieve an accuracy in beam polarization measurements that must be below 0.5%. This very high accuracy can be reached using polarized atomic hydrogen gas, stored in an ultra-cold magnetic trap, as the target for electron beam polarimetry based on Mo/ller scattering. Electron spin-polarized atomic hydrogen can be stored at high densities of 10{sup 16} cm{sup −2}, over relatively long time periods, in a high magnetic field (8T) and at low temperatures (0.3K). The gradient force splits the ground state of the hydrogen into four states with different energies. Atoms in the low energy states are trapped in the strong magnetic field region whereas the high energy states are repelled and pumped away. The physics of ultra-cold atomic hydrogen in magnetic traps and the status of the Mainz Hydro-Mo/ller project will be presented.

  3. Atomic mechanism of polarization-controlled surface reconstruction in ferroelectric thin films

    NASA Astrophysics Data System (ADS)

    Gao, Peng; Liu, Heng-Jui; Huang, Yen-Lin; Chu, Ying-Hao; Ishikawa, Ryo; Feng, Bin; Jiang, Ying; Shibata, Naoya; Wang, En-Ge; Ikuhara, Yuichi

    2016-04-01

    At the ferroelectric surface, the broken translational symmetry induced bound charge should significantly alter the local atomic configurations. Experimentally revealing the atomic structure of ferroelectric surface, however, is very challenging due to the strong spatial variety between nano-sized domains, and strong interactions between the polarization and other structural parameters. Here, we study surface structures of Pb(Zr0.2Ti0.8)O3 thin film by using the annular bright-field imaging. We find that six atomic layers with suppressed polarization and a charged 180° domain wall are at negatively poled surfaces, no reconstruction exists at positively poled surfaces, and seven atomic layers with suppressed polarization and a charged 90° domain wall exist at nominally neutral surfaces in ferroelastic domains. Our results provide critical insights into engineering ferroelectric thin films, fine grain ceramics and surface chemistry devices. The state-of-the-art methodology demonstrated here can greatly advance our understanding of surface science for oxides.

  4. Optical lattice polarization effects on magnetically induced optical atomic clock transitions

    SciTech Connect

    Taichenachev, A. V.; Yudin, V. I.; Oates, C. W.

    2007-08-15

    We derive the frequency shift for a forbidden optical transition J=0{yields}J{sup '}=0 caused by the simultaneous actions of an elliptically polarized lattice field and a static magnetic field. We find that a simple configuration of lattice and magnetic fields leads to a cancellation of this shift to first order in lattice intensity and magnetic field. In this geometry, the second-order lattice intensity shift can be minimized as well by use of optimal lattice polarization. Suppression of these shifts could considerably enhance the performance of the next generation of atomic clocks.

  5. H-atom ionization by elliptically polarized microwave fields: The overlap criterion

    SciTech Connect

    Sacha, K.; Zakrzewski, J.

    1997-07-01

    The threshold for H-atom ionization by elliptically polarized microwave fields is discussed within the classical-mechanics framework using the Chirikov overlap criterion. It is shown that the trends observed in the recent experiment [M. R. W. Bellermann {ital et al.} Phys. Rev. Lett. {bold 76}, 892 (1996)] are qualitatively reproduced by the theory; the origin of the remaining discrepancy is discussed. Increased stability of some orbits with respect to the perturbation due to the elliptically polarized microwaves has been related to vanishing widths of the corresponding resonance islands. Analytic Chirikov overlap prediction is compared with results of numerical simulations. {copyright} {ital 1997} {ital The American Physical Society}

  6. Coherent-population-trapping resonances with linearly polarized light for all-optical miniature atomic clocks

    SciTech Connect

    Zibrov, Sergei A.; Velichansky, Vladimir L.; Novikova, Irina; Phillips, David F.; Walsworth, Ronald L.; Zibrov, Alexander S.; Taichenachev, Alexey V.; Yudin, Valery I.

    2010-01-15

    We present a joint theoretical and experimental characterization of the coherent population trapping (CPT) resonance excited on the D{sub 1} line of {sup 87}Rb atoms by bichromatic linearly polarized laser light. We observe high-contrast transmission resonances (up to approx =25%), which makes this excitation scheme promising for miniature all-optical atomic clock applications. We also demonstrate cancellation of the first-order light shift by proper choice of the frequencies and relative intensities of the two laser-field components. Our theoretical predictions are in good agreement with the experimental results.

  7. Photoelectron momentum distributions of the hydrogen atom driven by multicycle elliptically polarized laser pulses

    NASA Astrophysics Data System (ADS)

    Murakami, Mitsuko; Chu, Shih-I.

    2016-02-01

    Photoelectron momentum distributions (PMDs) of the hydrogen atom driven by multicycle elliptically polarized strong laser fields are studied in detail, based on the numerical solution of the time-dependent Schrödinger equation and the Volkov wave propagation. Both short and long driving pulses of the 800-nm field are considered, as well as the ellipticity dependence, to describe the mechanism of symmetry breaking in the hydrogen-atom PMD. Moreover, we demonstrate that the value of a retardation angle in the longitudinal PMD can depend on the order of above-threshold ionization spectra.

  8. Coherent manipulation of spin-wave vector for polarization of photons in an atomic ensemble

    SciTech Connect

    Li Shujing; Xu Zhongxiao; Zheng Haiyan; Zhao Xingbo; Wu Yuelong; Wang Hai; Xie Changde; Peng Kunchi

    2011-10-15

    We experimentally demonstrate the manipulation of two orthogonal components of a spin wave in an atomic ensemble. Based on Raman two-photon transition and Larmor spin precession induced by magnetic field pulses, the coherent rotations between the two components of the spin wave are controllably achieved. Successively, the two manipulated spin-wave components are mapped into two orthogonal polarized optical emissions. By measuring Ramsey fringes of the retrieved optical signals, the {pi}/2-pulse fidelity of {approx}96% is obtained. The presented manipulation scheme can be used to build an arbitrary rotation for qubit operations in quantum information processing based on atomic ensembles.

  9. The spin polarized linear response from density functional theory: theory and application to atoms.

    PubMed

    Fias, Stijn; Boisdenghien, Zino; De Proft, Frank; Geerlings, Paul

    2014-11-14

    Within the context of spin polarized conceptual density functional theory, the spin polarized linear response functions are introduced both in the [N, N(s)] and [N(α), N(β)] representations. The mathematical relations between the spin polarized linear response functions in both representations are examined and an analytical expression for the spin polarized linear response functions in the [N(α), N(β)] representation is derived. The spin polarized linear response functions were calculated for all atoms up to and including argon. To simplify the plotting of our results, we integrated χ(r, r') to a quantity χ(r, r'), circumventing the θ and ϕ dependence. This allows us to plot and to investigate the periodicity throughout the first three rows in the periodic table within the two different representations. For the first time, χ(αβ)(r, r'), χ(βα)(r, r'), and χ(SS)(r, r') plots have been calculated and discussed. By integration of the spin polarized linear response functions, different components to the polarisability, α(αα), α(αβ), α(βα), and α(ββ) have been calculated. PMID:25399132

  10. The spin polarized linear response from density functional theory: Theory and application to atoms

    SciTech Connect

    Fias, Stijn Boisdenghien, Zino; De Proft, Frank; Geerlings, Paul

    2014-11-14

    Within the context of spin polarized conceptual density functional theory, the spin polarized linear response functions are introduced both in the [N, N{sub s}] and [N{sub α}, N{sub β}] representations. The mathematical relations between the spin polarized linear response functions in both representations are examined and an analytical expression for the spin polarized linear response functions in the [N{sub α}, N{sub β}] representation is derived. The spin polarized linear response functions were calculated for all atoms up to and including argon. To simplify the plotting of our results, we integrated χ(r, r′) to a quantity χ(r, r{sup ′}), circumventing the θ and ϕ dependence. This allows us to plot and to investigate the periodicity throughout the first three rows in the periodic table within the two different representations. For the first time, χ{sub αβ}(r, r{sup ′}), χ{sub βα}(r, r{sup ′}), and χ{sub SS}(r, r{sup ′}) plots have been calculated and discussed. By integration of the spin polarized linear response functions, different components to the polarisability, α{sub αα}, α{sub αβ}, α{sub βα}, and α{sub ββ} have been calculated.

  11. Magic polarization for optical trapping of atoms without Stark-induced dephasing.

    PubMed

    Kim, Huidong; Han, Hyok Sang; Cho, D

    2013-12-13

    We demonstrate that the differential ac-Stark shift of a Zeeman-sensitive ground hyperfine transition in an optical trap can be eliminated by using properly polarized trapping light. We use the vector polarizability of an alkali-metal atom to produce a polarization-dependent ac-Stark shift that resembles a Zeeman shift. We study a transition from the |2S1/2,F=2,mF=-2> to the |2S1/2,F=1,mF=-1> state of 7Li to observe 0.59±0.02  Hz linewidth with interrogation time of 2 s and 0.82±0.06  s coherence time of a superposition state. Implications of the narrow linewidth and the long coherence time for precision spectroscopy and quantum information processing using atoms in an optical lattice are discussed. PMID:24483653

  12. Magic Polarization for Optical Trapping of Atoms without Stark-Induced Dephasing

    NASA Astrophysics Data System (ADS)

    Kim, Huidong; Han, Hyok Sang; Cho, D.

    2013-12-01

    We demonstrate that the differential ac-Stark shift of a Zeeman-sensitive ground hyperfine transition in an optical trap can be eliminated by using properly polarized trapping light. We use the vector polarizability of an alkali-metal atom to produce a polarization-dependent ac-Stark shift that resembles a Zeeman shift. We study a transition from the |2S1/2,F=2,mF=-2⟩ to the |2S1/2,F=1,mF=-1⟩ state of Li7 to observe 0.59±0.02Hz linewidth with interrogation time of 2 s and 0.82±0.06s coherence time of a superposition state. Implications of the narrow linewidth and the long coherence time for precision spectroscopy and quantum information processing using atoms in an optical lattice are discussed.

  13. Photoionization of Synchrotron-Radiation-Excited Atoms: Separating Partial Cross Sections by Full Polarization Control

    SciTech Connect

    Aloiese, S.; Meyer, M.; Cubaynes, D.; Grum-Grzhimailo, A. N.

    2005-06-10

    Resonant atomic excitation by synchrotron radiation and subsequent ionization by a tunable dye laser is used to study the photoionization of short-lived Rydberg states in Xe. By combining circular and linear polarization of the synchrotron as well as of the laser photons the partial photoionization cross sections were separated in the region of overlapping autoionizing resonances of different symmetry and the parameters of the resonances were extracted.

  14. Polar atomic displacements in multiferroics observed via anomalous x-ray diffraction

    NASA Astrophysics Data System (ADS)

    Azimonte, C.; Granado, E.; Terashita, H.; Park, S.; Cheong, S.-W.

    2010-01-01

    The minute polar atomic displacements in multiferroics are shown to be within the reach of crystallography. A nonconventional methodology with anomalous x-ray diffraction is employed to investigate such displacements in DyMn2O5 with giant magnetoelectric coupling and two distinct Mn3+ and Mn4+ sites. Intensity differences of a selected Bragg reflection were measured as the direction of electric polarization is switched by a poling field. A significant differential effect, which is strongly enhanced at energies near and above the MnK edge, was observed near and below the ferroelectric transition temperature, Tc˜40K . The direct participation of ionic displacements in the ferroelectric polarization, particularly the Mn3+ sublattice, is demonstrated, dismissing a purely electronic mechanism for the multiferroicity.

  15. Polarization effects in the interaction between multi-level atoms and two optical fields

    NASA Astrophysics Data System (ADS)

    Colín-Rodríguez, R.; Flores-Mijangos, J.; Hernández-Gómez, S.; Jáuregui, R.; López-Hernández, O.; Mojica-Casique, C.; Ponciano-Ojeda, F.; Ramírez-Martínez, F.; Sahagún, D.; Volke-Sepúlveda, K.; Jiménez-Mier, J.

    2015-06-01

    Polarized velocity selective spectra for rubidium atoms in a room temperature cell are presented. The experiments were performed in the lambda configuration (D2 manifold) and in the 5s\\to 5{{p}3/2}\\to 5{{d}j} ladder configuration. For the lambda configuration the effect of the probe beam intensity in the absorption and polarization spectra are compared with results of a rate equation approximation. Good overall agreement between experiment and theory is found. The results indicate different saturation rates for each of the atomic transitions. Distinctive polarization signals with hyperfine-resolved components are found for the ladder 5{{d}3/2} and 5{{d}5/2} upper states. Fluorescence detection of the 420 nm that results from the second step in the cascade decay 5{{d}j}\\to 6{{p}{{j\\prime }}}\\to 5s was used in the ladder experiments. This fluorescence was also used for the detection of the 5{{p}3/2}\\to 6{{p}3/2} electric dipole forbidden transition in atomic rubidium that occurs at 911 nm. The 6{{p}3/2} hyperfine structure was resolved in this continuous wave, non-dipole excitation.

  16. High resolution photofragment translational spectroscopy of the near UV photolysis of indole: dissociation via the 1pi sigma* state.

    PubMed

    Nix, M G D; Devine, A L; Cronin, B; Ashfold, M N R

    2006-06-14

    The fragmentation dynamics of indole molecules following excitation at 193.3 nm, and at a number of different wavelengths in the range 240 < or = lambda(phot) < or = 286 nm, have been investigated by H Rydberg atom photofragment translational spectroscopy. The longer wavelength measurements have been complemented by measurements of excitation spectra for forming parent and fragment ions by two (or more) photon ionisation processes. Analysis identifies at least three distinct contributions to the observed H atom yield, two of which are attributable to dissociation of indole following radiationless transfer from the 1pi pi* excited states (traditionally labelled 1L(b) and 1L(a)) prepared by UV single photon absorption. The structured channel evident in total kinetic energy release (TKER) spectra recorded at lambda(phot) < or = 263 nm is rationalised in terms of N-H bond fission following initial pi* <-- pi excitation and subsequent coupling to the 1pi sigma* potential energy surface via a conical intersection between the respective surfaces--thereby validating recent theoretical predictions regarding the importance of this process (Sobolewski et al., Phys. Chem. Chem. Phys., 2002, 4, 1093). Analysis provides an upper limit for the N-H bond strength in indole: D0(H-indolyl) < or = 31,900 cm(-1). Unimolecular decay of highly vibrationally excited ground state molecules formed by internal conversion from the initially prepared 1pi pi* states is a source of (slow) H atoms but their contribution to the TKER spectra measured in the present work is dwarfed by that from H atoms generated by one or more (unintended but unavoidable) multiphoton processes. PMID:16738714

  17. Atomic scattering spectroscopy for determination of the polarity of semipolar AlN grown on ZnO

    SciTech Connect

    Kobayashi, Atsushi; Ohta, Jitsuo; Ueno, Kohei; Oshima, Masaharu; Fujioka, Hiroshi

    2013-11-04

    Determination of the polarity of insulating semipolar AlN layers was achieved via atomic scattering spectroscopy. The back scattering of neutralized He atoms on AlN surfaces revealed the atomic alignment of the topmost layers of semipolar AlN and the ZnO substrate. Pole figures of the scattering intensity were used to readily determine the polarity of these wurtzite-type semipolar materials. In addition, we found that +R-plane AlN epitaxially grows on −R-plane ZnO, indicating that the polarity flips at the semipolar AlN/ZnO interface. This polarity flipping is possibly explained by the appearance of −c and m-faces on the −R ZnO surfaces, which was also revealed by atomic scattering spectroscopy.

  18. Fast, high-fidelity, all-optical and dynamically-controlled polarization gate using room-temperature atomic vapor

    SciTech Connect

    Li, Runbing; Zhu, Chengjie; Deng, L.; Hagley, E. W.

    2014-10-20

    We demonstrate a fast, all-optical polarization gate in a room-temperature atomic medium. Using a Polarization-Selective-Kerr-Phase-Shift (PSKPS) technique, we selectively write a π phase shift to one circularly-polarized component of a linearly-polarized input signal field. The output signal field maintains its original strength but acquires a 90° linear polarization rotation, demonstrating fast, high-fidelity, dynamically-controlled polarization gate operation. The intensity of the polarization-switching field used in this PKSPK-based polarization gate operation is only 2 mW/cm{sup 2}, which would be equivalent to 0.5 nW of light power (λ = 800 nm) confined in a typical commercial photonic hollow-core fiber. This development opens a realm of possibilities for potential future extremely low light level telecommunication and information processing systems.

  19. Nonadiabatic theory of strong-field atomic effects under elliptical polarization

    SciTech Connect

    Wang Xu; Eberly, J. H.

    2012-12-14

    Elliptically polarized laser fields provide a new channel for access to strong-field processes that are either suppressed or not present under linear polarization. Quantum theory is mostly unavailable for their analysis, and we report here results of a systematic study based on a classical ensemble theory with solution of the relevant ab inito time-dependent Newton equations for selected model atoms. The study's approach is necessarily nonadiabatic, as it follows individual electron trajectories leading to single, double, and triple ionizations. Of particular interest are new results bearing on open questions concerning experimental reports of unexplained species dependences as well as double-electron release times that are badly matched by a conventional adiabatic quantum tunneling theory. We also report the first analysis of electron trajectories for sequential and non-sequential triple ionization.

  20. Photoelectron angular distributions from polarized Ne{sup *} atoms near threshold

    SciTech Connect

    O'Keeffe, P.; Bolognesi, P.; Mihelic, A.; Moise, A.; Richter, R.; Cautero, G.; Stebel, L.; Sergo, R.; Pravica, L.; Ovcharenko, E.; Decleva, P.; Avaldi, L.

    2010-11-15

    Photoelectron distributions of the polarized 2p{sup 5}3d Rydberg states of neon have been studied with a newly built velocity map imaging analyzer. The atoms were polarized by absorption of synchrotron radiation and ionized by an infrared laser. The asymmetry parameters {beta}{sub 2} and {beta}{sub 4} characterizing two-photon resonant ionization have been extracted from the measured images and compared with the results of a quantum defect treatment. To achieve a good theoretical description of the data, it is necessary to take into account the dependence of the dipole transition matrix elements and phases of the partial waves on the angular momentum quantum numbers pertaining to various continuum channels.

  1. Exploring conical intersections through high resolution photofragment translational spectroscopy

    NASA Astrophysics Data System (ADS)

    Ashfold, Michael

    2007-03-01

    High resolution measurements of the kinetic energies of H atom fragments formed during UV photolysis of gas phase imidazole, [1,2] pyrrole, [3] phenol [4] and thiophenol molecules show that: (i) X-H (X = N, O, S) bond fission is an important non-radiative decay process from the ^1πσ* excited states in each of these molecules, and (ii) that the respective co-fragments (imidazolyl, pyrrolyl, phenoxyl and thiophenoxyl) are formed in very limited sub-sets of their available vibrational states. Identification of these product states yields uniquely detailed insights into the vibronic couplings involved in the photo-induced evolution from parent molecule to ultimate fragments. [1] M.N.R. Ashfold, B. Cronin, A.L. Devine, R.N. Dixon and M.G.D. Nix, Science (2006), 312, 1637. [2] A.L. Devine, B. Cronin, M.G.D. Nix and M.N.R. Ashfold, J. Chem. Phys. (in press). [3] B. Cronin, M.G.D. Nix, R.H. Qadiri and M.N.R. Ashfold, Phys. Chem. Chem. Phys. (2004), 6, 5031. [4] M.G.D. Nix, A.L. Devine, B. Cronin, R.N. Dixon and M.N.R. Ashfold, J. Chem. Phys. (2006), 125, 133318.

  2. Resonance overlap criterion for H atom ionization by circularly polarized microwave fields

    SciTech Connect

    Sacha, K.; Zakrzewski, J.

    1997-01-01

    The threshold for H atom ionization by circularly polarized microwave fields is discussed within the classical mechanics framework for high microwave frequencies. The Chirikov resonance overlap criterion predictions are compared with estimates obtained adopting the renormalization method. It is shown that the ionization threshold is highly sensitive to the helicity of microwaves. Among all possible initial electronic orbits, those of medium eccentricity are the first to ionize. The results obtained indicate that collisions with the nucleus play a negligible role for the onset of ionization. {copyright} {ital 1997} {ital The American Physical Society}

  3. Measuring the spin polarization of alkali-metal atoms using nuclear magnetic resonance frequency shifts of noble gases

    NASA Astrophysics Data System (ADS)

    Liu, X. H.; Luo, H.; Qu, T. L.; Yang, K. Y.; Ding, Z. C.

    2015-10-01

    We report a novel method of measuring the spin polarization of alkali-metal atoms by detecting the NMR frequency shifts of noble gases. We calculated the profile of 87Rb D1 line absorption cross sections. We then measured the absorption profile of the sample cell, from which we calculated the 87Rb number densities at different temperatures. Then we measured the frequency shifts resulted from the spin polarization of the 87Rb atoms and calculated its polarization degrees at different temperatures. The behavior of frequency shifts versus temperature in experiment was consistent with theoretical calculation, which may be used as compensative signal for the NMRG closed-loop control system.

  4. Electron impact polarization of atomic spectral lines. I - A general theoretical scheme

    NASA Technical Reports Server (NTRS)

    Fineschi, Silvano; Degl'innocenti, Egidio L.

    1992-01-01

    A suitable theoretical scheme able to describe, in a wide variety of astrophysical situations, the phenomenon of atomic line polarization by electron impact is developed. Starting from the general principles of quantum mechanics and assuming the Born approximation, the rate equations for the density matrix elements of a multilevel atomic system, interacting with a nonrelativistic electron beam having any kind of angular distribution, are derived in full generality. The resulting theory generalizes the previous ones by accounting for the collisional rates and the cross sections concerning both inelastic and superelastic collisions (in any geometrical situation), and, moreover, by taking into account the coherences among Zeeman sublevels split by a magnetic field. As an example of particular relevance, the general formulas derived in the first sections of the paper are subsequently particularized to the case of the electric dipole interaction.

  5. Dielectronic Recombination, Autoionization and Non-Adiabatic Core Polarization of Rydberg Two-Electron Atoms

    NASA Astrophysics Data System (ADS)

    Nunkaew, Jirakan

    In this dissertation, I study the structure and dynamics of Rydberg two-electron atoms. Specifically, I study the core polarization effect of the Rydberg electron on the ground state ion of strontium and the autoionization of barium atoms in an external static field in the low field regime. The autoionization studies show that it is possible to measure the contribution to dielectronic recombination (DR) of energetically unresolved high ℓ states by measuring the recombination rate as a function of electric field. I also present the experimental observation that the ejected electrons from autoionizing states in an electric field have a directional preference that depends on the orientation of the Rydberg Stark state wavefunctions. Finally, I present the spectroscopy of the Stark autoionizing states in the low field regime using a high resolution dye-amplified diode laser.

  6. Improved sliced velocity map imaging apparatus optimized for H photofragments.

    PubMed

    Ryazanov, Mikhail; Reisler, Hanna

    2013-04-14

    Time-sliced velocity map imaging (SVMI), a high-resolution method for measuring kinetic energy distributions of products in scattering and photodissociation reactions, is challenging to implement for atomic hydrogen products. We describe an ion optics design aimed at achieving SVMI of H fragments in a broad range of kinetic energies (KE), from a fraction of an electronvolt to a few electronvolts. In order to enable consistently thin slicing for any imaged KE range, an additional electrostatic lens is introduced in the drift region for radial magnification control without affecting temporal stretching of the ion cloud. Time slices of ∼5 ns out of a cloud stretched to ⩾50 ns are used. An accelerator region with variable dimensions (using multiple electrodes) is employed for better optimization of radial and temporal space focusing characteristics at each magnification level. The implemented system was successfully tested by recording images of H fragments from the photodissociation of HBr, H2S, and the CH2OH radical, with kinetic energies ranging from <0.4 eV to >3 eV. It demonstrated KE resolution ≲1%-2%, similar to that obtained in traditional velocity map imaging followed by reconstruction, and to KE resolution achieved previously in SVMI of heavier products. We expect it to perform just as well up to at least 6 eV of kinetic energy. The tests showed that numerical simulations of the electric fields and ion trajectories in the system, used for optimization of the design and operating parameters, provide an accurate and reliable description of all aspects of system performance. This offers the advantage of selecting the best operating conditions in each measurement without the need for additional calibration experiments. PMID:24981528

  7. Improved sliced velocity map imaging apparatus optimized for H photofragments

    SciTech Connect

    Ryazanov, Mikhail; Reisler, Hanna

    2013-04-14

    Time-sliced velocity map imaging (SVMI), a high-resolution method for measuring kinetic energy distributions of products in scattering and photodissociation reactions, is challenging to implement for atomic hydrogen products. We describe an ion optics design aimed at achieving SVMI of H fragments in a broad range of kinetic energies (KE), from a fraction of an electronvolt to a few electronvolts. In order to enable consistently thin slicing for any imaged KE range, an additional electrostatic lens is introduced in the drift region for radial magnification control without affecting temporal stretching of the ion cloud. Time slices of {approx}5 ns out of a cloud stretched to Greater-Than-Or-Slanted-Equal-To 50 ns are used. An accelerator region with variable dimensions (using multiple electrodes) is employed for better optimization of radial and temporal space focusing characteristics at each magnification level. The implemented system was successfully tested by recording images of H fragments from the photodissociation of HBr, H{sub 2}S, and the CH{sub 2}OH radical, with kinetic energies ranging from <0.4 eV to >3 eV. It demonstrated KE resolution Less-Than-Or-Equivalent-To 1%-2%, similar to that obtained in traditional velocity map imaging followed by reconstruction, and to KE resolution achieved previously in SVMI of heavier products. We expect it to perform just as well up to at least 6 eV of kinetic energy. The tests showed that numerical simulations of the electric fields and ion trajectories in the system, used for optimization of the design and operating parameters, provide an accurate and reliable description of all aspects of system performance. This offers the advantage of selecting the best operating conditions in each measurement without the need for additional calibration experiments.

  8. Topological phases in atoms and molecules in spin-polarized electron scattering

    NASA Astrophysics Data System (ADS)

    Williams, James; Pravica, Luka; Samarin, Sergey; Kathi, Sudarshan; Guagliardo, Paul; CentreAtomic, Molecular; Surface Physics Team

    2013-05-01

    Observations of spin-polarized electron impact excitation of zinc atoms, ionization of helium atoms and dissociative excitation of molecules indicate a topological phase. The parallel transport of the spin vector gives rise to an effective `monopole' magnetic field and an apparent spin-orbit interaction. In excitation, the Stokes parameters of radiated photons show alignment and orientation. Excitation of a superposition of 2s and 2p states on atomic hydrogen in an external electric field show beats in Lyman alpha radiation as predicted for a circular vortex. Ionization of helium atoms show minima in (e,2e) angular and energy differential cross sections associated with a linear vortex (Macek, Feagin). Exchange dissociative excitation of methane shows radiated photons from a Jahn-Teller ``avoided crossing'' of potential energy curves (Mead and Truhlar). The observations are consistent with fundamental principles that a gauge-invariant quantity is potentially a physical observable and the topology of a ring indicates a magnetic-flux line enclosed by the ring is equivalent to a vortex line. Funding was received from the Australian Research Council and The University of Western Australia.

  9. Optimal densities of alkali metal atoms in an optically pumped K-Rb hybrid atomic magnetometer considering the spatial distribution of spin polarization.

    PubMed

    Ito, Yosuke; Sato, Daichi; Kamada, Keigo; Kobayashi, Tetsuo

    2016-07-11

    An optically pumped K-Rb hybrid atomic magnetometer can be a useful tool for biomagnetic measurements due to the high spatial homogeneity of its sensor property inside a cell. However, because the property varies depending on the densities of potassium and rubidium atoms, optimization of the densities is essential. In this study, by using the Bloch equations of K and Rb and considering the spatial distribution of the spin polarization, we confirmed that the calculation results of spin polarization behavior are in good agreement with the experimental data. Using our model, we calculated the spatial distribution of the spin polarization and found that the optimal density of K atoms is 3 × 1019 m-3 and the optimal density ratio is nK/nRb ~ 400 to maximize the output signal and enhance spatial homogeneity of the sensor property. PMID:27410815

  10. Atomic origin of the spin-polarization of the Co2FeAl Heusler compound

    NASA Astrophysics Data System (ADS)

    Liang, Jaw-Yeu; Lam, Tu-Ngoc; Lin, Yan-Cheng; Chang, Shu-Jui; Lin, Hong-Ji; Tseng, Yuan-Chieh

    2016-02-01

    Using synchrotron x-ray techniques, we studied the Co2FeAl spin-polarization state that generates the half-metallicity of the compound during an A2 (low-spin)  →  B2 (high-spin) phase transition. Given the advantage of element specificity of x-ray techniques, we could fingerprint the structural and magnetic cross-reactions between Co and Fe within a complex Co2FeAl structure deposited on a MgO (0 0 1) substrate. X-ray diffraction and extended x-ray absorption fine structure investigations determined that the Co atoms preferably populate the (1/4,1/4,1/4) and (3/4,3/4,3/4) sites during the development of the B2 phase. X-ray magnetic spectroscopy showed that although the two magnetic elements were ferromagnetically coupled, they interacted in a competing manner via a charge-transfer effect, which enhanced Co spin polarization at the expense of Fe spin polarization during the phase transition. This means that the spin-polarization of Co2FeAl was electronically dominated by Fe in A2 whereas the charge transfer turned the dominance to Co upon B2 formation. Helicity-dependent x-ray absorption spectra also revealed that only the minority state of Co/Fe was involved in the charge-transfer effect whereas the majority state was independent of it. Despite an overall increase of Co2FeAl magnetization, the charge-transfer effect created an undesired trade-off during the Co-Fe exchange interactions, because of the presence of twice as many X sites (Co) as Y sites (Fe) in the Heusler X 2 YZ formula. This suggests that the spin-polarization of Co2FeAl is unfortunately regulated by compromising the enhanced X (Co) sites and the suppressed Y (Fe) sites, irrespective of the development of the previously known high-spin-polarization phase of B2. This finding provides a possible cause for the limited half-metallicity of Co2FeAl discovered recently. Electronic tuning between the X and Y sites is necessary to further increase the spin-polarization, and likely the half

  11. Polarized electron correlations near auto-ionizing states of zinc atoms

    NASA Astrophysics Data System (ADS)

    Williams, James; Pravica, Luka; Samarin, Sergey

    2015-09-01

    Multi-electron metal atoms find new applications in diverse structures with spin and momentum-dependent properties having significance in determining material functionalities. Electron correlations effects are determined from scattering kinematics of spin-polarized electrons exciting zinc atoms near autoionizing states up to 16 eV. Previous studies of the 4p 3 , 1P1 , 4 d,5 d,6d3D1 , 2 , 3 and 4 d,5d1D1 excited states observed photon decay intensities and scattered electron energies and angles in the energy region of the 3d94s24 p autoionizing states up to 12 eV. Strong electron correlations and active roles of 3 d electrons were evident. Our observations of the 53S excited state for electron energies up to 16 eV show dominant 3 d core-excited negative-ion resonances and strong Post-Collision Interaction (PCI). For low energies of scattered and ejected electrons, after near-threshold excitation of the 3d94s24 p autoionizing states, a large transfer of orbital angular momentum is evident. Results include angular differential elastic scattering and excitation functions, ``integrated'' Stokes polarization parameters and spin up/down asymmetries indicating spin-orbit interaction and electron exchange effects. School of Physics

  12. Effects of local sample bending on atom positions and polarization mapping in HAADF-STEM images

    NASA Astrophysics Data System (ADS)

    Wang, Zhen; Guo, Hangwen; Chen, Lina; Plummer, E. W.; Zhang, Jiandi; Tao, Jing; Wu, Lijun; Zhu, Yimei

    Characterization of the structural distortion/reconstruction in the transition-metal oxide heterostructures play an important role in understanding their novel properties. In recent years, high-angle annular dark field (HAADF) in scanning transmission electron microscopy (STEM) has become a powerful technique to determine local atomic arrangements, particularly near interfaces and boundaries. However, sample bending, especially near the edge of a thin specimen, is often introduced during the TEM sample preparation process. Our recent studies reveal that small sample bending can affect significantly the measurement of atom positions in HAADF-STEM image as a result of channeling effect of the incident electron beam. Here we take SrTiO3 (STO) as an example to show how to remove sample bending induced artifact from its intrinsic structural distortions. A polar-related artifact in STO at different bending angles were reveled both in our experiments and imaging simulation. This artifact can be removed successfully by quantitative comparing experimental with simulated HAADF-STEM images under the same imaging condition. The bending angle and thickness of the sample can be determined using convergent beam electron diffraction. Our study provide a useful guidance for removing the sample bending-induced artifact in STEM images for the studies of local lattice structures, polarization and distortion of complex materials.

  13. Valley polarization and coherence in atomically thin tungsten disulfide via optical spectroscopy

    NASA Astrophysics Data System (ADS)

    Zhu, Bairen; Zeng, Hualing; Dai, Junfeng; Gong, Zhirui; Cui, Xiaodong

    Atomically thin group-VI transition metal dichalcogenides (TMDC) has been emerging as a family of intrinsic 2-dimensional crystals with a sizeable bandgap, opening a potential avenue for ultimate electronics and optoelectronics. Besides, the characteristic structural inversion symmetry breaking in monolayers leads to non-zero but contrasting Berry curvatures and orbital magnetic moments at K/K' valleys. These features provide an opportunity to manipulate electrons' additional internal degrees of freedom, namely the valley degree of freedom, making monolayer TMDC a promising candidate for the conceptual valleytronics. Here, our experimental approach on valley dependent circular dichroism in monolayer and bilayer WS2 via optical spectroscopy are elaborated. Consequently, the polarization of photoluminescence inherits that of excitations, circularly and linearly polarized, confirming the valley dependent selectivity rule. However, the valley polarization and valley coherence in bilayer WS2 owing to the coupling of spin, valley and layer degrees of freedom, are anomalously robust compared with monolayer WS2. We propose potential mechanisms of the anomalous behavior in WS2 bilayers.

  14. Controlled polarization of two-dimensional quantum turbulence in atomic Bose-Einstein condensates

    NASA Astrophysics Data System (ADS)

    Cidrim, A.; dos Santos, F. E. A.; Galantucci, L.; Bagnato, V. S.; Barenghi, C. F.

    2016-03-01

    We propose a scheme for generating two-dimensional turbulence in harmonically trapped atomic condensates with the novelty of controlling the polarization (net rotation) of the turbulence. Our scheme is based on an initial giant (multicharged) vortex which induces a large-scale circular flow. Two thin obstacles, created by blue-detuned laser beams, speed up the decay of the giant vortex into many singly quantized vortices of the same circulation; at the same time, vortex-antivortex pairs are created by the decaying circular flow past the obstacles. Rotation of the obstacles against the circular flow controls the relative proportion of positive and negative vortices, from the limit of strongly anisotropic turbulence (almost all vortices having the same sign) to that of isotropic turbulence (equal number of vortices and antivortices). Using this scheme, we numerically study the decay of two-dimensional quantum turbulence as a function of the polarization. Finally, we present a model for the decay rate of the vortex number which fits our numerical experiment curves, with the novelty of taking into account polarization time dependence.

  15. Atomic structure of defects in GaN:Mg grown with Ga polarity

    SciTech Connect

    Liliental-Weber, Z.; Tomaszewicz, T.; Zakharov, D.; Jasinski, J.; O'Keefe, M.A.; Hautakangas, S.; Laakso, A.; Saarinen, K.

    2003-11-25

    Electron microscope phase images, produced by direct reconstruction of the scattered electron wave from a focal series of high-resolution images, were used to determine the nature of defects formed in GaN:Mg crystals. We studied bulk crystals grown from dilute solutions of atomic nitrogen in liquid gallium at high pressure and thin films grown by the MOCVD method. All the crystals were grown with Ga-polarity. In both types of samples the majority of defects were three dimensional Mg-rich hexagonal pyramids with bases on the (0001) plane and six walls on {l_brace}11{und 2}3{r_brace} planes seen in cross-section as triangulars. Some other defects appear in cross-section as trapezoidal (rectangular) defects as a result of presence of truncated pyramids. Both type of defects have hollow centers. They are decorated by Mg on all six side walls and a base. The GaN which grows inside on the defect walls shows polarity inversion. It is shown that change of polarity starts from the defect tip and propagates to the base, and that the stacking sequence changes from ab in the matrix to bc inside the defect. Exchange of the Ga sublattice with the N sublattice within the defect leads to 0.6 {+-} 0.2{angstrom} displacement between Ga sublattices outside and inside the defects. It is proposed that lateral overgrowth of the cavities formed within the defect takes place to restore matrix polarity on the defect base.

  16. Role of high-lying electronic states on the angular distribution of photofragments in multiphoton dissociation of D{sub 2}{sup +} by intense laser fields

    SciTech Connect

    Sen, Sanjay; Dutta, Bibhas; Bhattacharyya, S. S.; Saha, Samir

    2003-05-01

    We have theoretically investigated the role of high lying electronic states 2p{pi}{sub u} and 3d{sigma}{sub g} on multiphoton dissociation of D{sub 2}{sup +} from initial vibrational-rotational levels v{sub i}=4,5 and J{sub i}=0,1 by linearly polarized light with wavelength 400 nm and intensity 3x10{sup 13} W/cm{sup 2}. We have found that for initial level v{sub i}=4 and J{sub i}=1, a considerable number of photofragments is ejected perpendicular to the polarization direction of the laser field. It is shown that the perpendicular dissociation is due to the (net) four-photon absorption of the ground 1s{sigma}{sub g} state to the 3d{sigma}{sub g} state through the intermediate five-photon coupling of the 1s{sigma}{sub g} and 2p{pi}{sub u} states at intense laser field with high frequency. Our computed value of the emission of D{sup +} ions in the perpendicular direction to that in the parallel direction of the laser polarization reasonably agrees with the recent experimental result of Chin and co-workers at the same laser parameters [Phys. Rev. A 62, 042708 (2000)].

  17. Revisiting the integrated infrared intensities and atomic polar tensors of the boron trihalides.

    PubMed

    Richter, Wagner E; Bruns, Roy E

    2016-07-01

    Integrated infrared intensities obtained from spectra of the Pacific Northwest National Laboratory (PNNL) database are reported for BF3, BCl3 and BBr3. The BF3 and BCl3 intensities are compared with values reported much earlier whereas the asymmetric BBr3 stretching intensity is reported for the first time. Although agreement is good for the BF3 intensities, the result from the PNNL spectra for the asymmetric BCl3 stretching vibration is about three times larger than the one reported earlier. The intensities obtained from the PNNL spectra are in excellent agreement with results from QCISD/cc-pVTZ quantum chemical calculations having an rms error of only 32.9cm(-1) or 5.9% of the average intensity. Revised experimental atomic polar tensors and GAPT charges are reported for all these molecules. PMID:27092735

  18. Revisiting the integrated infrared intensities and atomic polar tensors of the boron trihalides

    NASA Astrophysics Data System (ADS)

    Richter, Wagner E.; Bruns, Roy E.

    2016-07-01

    Integrated infrared intensities obtained from spectra of the Pacific Northwest National Laboratory (PNNL) database are reported for BF3, BCl3 and BBr3. The BF3 and BCl3 intensities are compared with values reported much earlier whereas the asymmetric BBr3 stretching intensity is reported for the first time. Although agreement is good for the BF3 intensities, the result from the PNNL spectra for the asymmetric BCl3 stretching vibration is about three times larger than the one reported earlier. The intensities obtained from the PNNL spectra are in excellent agreement with results from QCISD/cc-pVTZ quantum chemical calculations having an rms error of only 32.9 cm- 1 or 5.9% of the average intensity. Revised experimental atomic polar tensors and GAPT charges are reported for all these molecules.

  19. Computational efficiency improvement with Wigner rotation technique in studying atoms in intense few-cycle circularly polarized pulses.

    PubMed

    Yuan, Minghu; Lü, Rui; Feng, Liqiang; Chu, Tianshu

    2014-02-21

    We show that by introducing Wigner rotation technique into the solution of time-dependent Schrödinger equation in length gauge, computational efficiency can be greatly improved in describing atoms in intense few-cycle circularly polarized laser pulses. The methodology with Wigner rotation technique underlying our openMP parallel computational code for circularly polarized laser pulses is described. Results of test calculations to investigate the scaling property of the computational code with the number of the electronic angular basis function l as well as the strong field phenomena are presented and discussed for the hydrogen atom. PMID:24559339

  20. Computational efficiency improvement with Wigner rotation technique in studying atoms in intense few-cycle circularly polarized pulses

    SciTech Connect

    Yuan, Minghu; Feng, Liqiang; Lü, Rui; Chu, Tianshu E-mail: tschu008@163.com

    2014-02-21

    We show that by introducing Wigner rotation technique into the solution of time-dependent Schrödinger equation in length gauge, computational efficiency can be greatly improved in describing atoms in intense few-cycle circularly polarized laser pulses. The methodology with Wigner rotation technique underlying our openMP parallel computational code for circularly polarized laser pulses is described. Results of test calculations to investigate the scaling property of the computational code with the number of the electronic angular basis function l as well as the strong field phenomena are presented and discussed for the hydrogen atom.

  1. Tailoring polarity in a layered nickelate with single atomic layer control

    NASA Astrophysics Data System (ADS)

    Bhattacharya, Anand; Nelson-Cheeseman, Brittany; Zhou, Hua; Balachandran, Prasanna; Fabbris, Gilberto; Hoffman, Jason; Haskel, Daniel; Rondinelli, James

    2014-03-01

    Many of the 3d transition metal oxides share a common structural MO6 building unit--a central transition metal (TM) cation octahedrally coordinated with oxygen nearest neighbors. The electronic states in these materials can be modified by tailoring the M-O bonds, which typically include the application of epitaxial strain in thin films, or pressure and isovalent cation substitution in bulk samples. Here, we present a new route to tailor the M-O bonds without changes to the strain state or stoichiometry in two-dimensional perovskite nickelate (n =1 in the Ruddlesden Popper series). We do this by tailoring the dipolar electrostatic interactions at the unit cell level in nominally non-polar LaSrNiO4 via single atomic layer-by-layer synthesis using oxide-MBE. We reconstruct the response of the crystal lattice to the induced polarity using a x-ray phase retrieval technique (COBRA). We find that the response of the O anions to the resulting local electric fields distorts the M-O bonds, being largest for the apical oxygens (Oap) . It also alters the Ni valence.

  2. Selective detection of angular-momentum-polarized Auger electrons by atomic stereography.

    PubMed

    Matsui, Fumihiko; Fujita, Masayoshi; Ohta, Takuya; Maejima, Naoyuki; Matsui, Hirosuke; Nishikawa, Hiroaki; Matsushita, Tomohiro; Daimon, Hiroshi

    2015-01-01

    When a core level is excited by circularly polarized light, the angular momentum of light is transferred to the emitted photoelectron, which can be confirmed by the parallax shift of the forward focusing peak (FFP) direction in a stereograph of atomic arrangement. No angular momentum has been believed to be transferred to normal Auger electrons resulting from the decay process filling core hole after photoelectron ejection. We succeeded in detecting a non-negligible circular dichroism contrast in a normal Auger electron diffraction from a nonmagnetic Cu(001) surface far off from the absorption threshold. Moreover, we detected angular-momentum-polarized Cu L(3)M(4,5)M(4,5) Auger electrons at the L(3) absorption threshold, where the excited core electron is trapped at the conduction band. From the kinetic energy dependence of the Auger electron FFP parallax shift, we found that the angular momentum is transferred to the Auger electron most effectively in the case of the (1)S(0) two-hole creation. PMID:25615477

  3. Sensitive determination of the spin polarization of optically pumped alkali-metal atoms using near-resonant light.

    PubMed

    Ding, Zhichao; Long, Xingwu; Yuan, Jie; Fan, Zhenfang; Luo, Hui

    2016-01-01

    A new method to measure the spin polarization of optically pumped alkali-metal atoms is demonstrated. Unlike the conventional method using far-detuned probe light, the near-resonant light with two specific frequencies was chosen. Because the Faraday rotation angle of this approach can be two orders of magnitude greater than that with the conventional method, this approach is more sensitive to the spin polarization. Based on the results of the experimental scheme, the spin polarization measurements are found to be in good agreement with the theoretical predictions, thereby demonstrating the feasibility of this approach. PMID:27595707

  4. Sensitive determination of the spin polarization of optically pumped alkali-metal atoms using near-resonant light

    PubMed Central

    Ding, Zhichao; Long, Xingwu; Yuan, Jie; Fan, Zhenfang; Luo, Hui

    2016-01-01

    A new method to measure the spin polarization of optically pumped alkali-metal atoms is demonstrated. Unlike the conventional method using far-detuned probe light, the near-resonant light with two specific frequencies was chosen. Because the Faraday rotation angle of this approach can be two orders of magnitude greater than that with the conventional method, this approach is more sensitive to the spin polarization. Based on the results of the experimental scheme, the spin polarization measurements are found to be in good agreement with the theoretical predictions, thereby demonstrating the feasibility of this approach. PMID:27595707

  5. ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS: Selective Deflection of Polarized Light Via Coherently Driven Four-Level Atoms in a Double-Λ Configuration

    NASA Astrophysics Data System (ADS)

    Guo, Yu

    2010-05-01

    We study the interaction of a weak probe field, having two circular polarized components, i.e., σ- and σ+ polarization, with an optically dense medium of four-level atoms in a double-Λ configuration, which is mediated by the electromagnetically induced transparency with a polarized control light with spatially inhomogeneous profile. We analyse the deflection of the polarized probe light and we find that we can selectively determine which circular component will be deflected after the polarized probe light enters the atom medium via adjusting the polarization and detuning of the control field.

  6. Atomic scale imaging of competing polar states in a Ruddlesden-Popper layered oxide.

    PubMed

    Stone, Greg; Ophus, Colin; Birol, Turan; Ciston, Jim; Lee, Che-Hui; Wang, Ke; Fennie, Craig J; Schlom, Darrell G; Alem, Nasim; Gopalan, Venkatraman

    2016-01-01

    Layered complex oxides offer an unusually rich materials platform for emergent phenomena through many built-in design knobs such as varied topologies, chemical ordering schemes and geometric tuning of the structure. A multitude of polar phases are predicted to compete in Ruddlesden-Popper (RP), An+1BnO3n+1, thin films by tuning layer dimension (n) and strain; however, direct atomic-scale evidence for such competing states is currently absent. Using aberration-corrected scanning transmission electron microscopy with sub-Ångstrom resolution in Srn+1TinO3n+1 thin films, we demonstrate the coexistence of antiferroelectric, ferroelectric and new ordered and low-symmetry phases. We also directly image the atomic rumpling of the rock salt layer, a critical feature in RP structures that is responsible for the competing phases; exceptional quantitative agreement between electron microscopy and density functional theory is demonstrated. The study shows that layered topologies can enable multifunctionality through highly competitive phases exhibiting diverse phenomena in a single structure. PMID:27578622

  7. Development of Two-Photon Pump Polarization Spectroscopy Probe Technique Tpp-Psp for Measurements of Atomic Hydrogen .

    NASA Astrophysics Data System (ADS)

    Satija, Aman; Lucht, Robert P.

    2015-06-01

    Atomic hydrogen (H) is a key radical in combustion and plasmas. Accurate knowledge of its concentration can be used to better understand transient phenomenon such as ignition and extinction in combustion environments. Laser induced polarization spectroscopy is a spatially resolved absorption technique which we have adapted for quantitative measurements of H atom. This adaptation is called two-photon pump, polarization spectroscopy probe technique (TPP-PSP) and it has been implemented using two different laser excitation schemes. The first scheme involves the two-photon excitation of 1S-2S transitions using a linearly polarized 243-nm beam. An anisotropy is created amongst Zeeman states in 2S-3P levels using a circularly polarized 656-nm pump beam. This anisotropy rotates the polarization of a weak, linearly polarized probe beam at 656 nm. As a result, the weak probe beam "leaks" past an analyzer in the detection channel and is measured using a PMT. This signal can be related to H atom density in the probe volume. The laser beams were created by optical parametric generation followed by multiple pulse dye amplification stages. This resulted in narrow linewidth beams which could be scanned in frequency domain and varied in energy. This allowed us to systematically investigate saturation and Stark effect in 2S-3P transitions with the goal of developing a quantitative H atom measurement technique. The second scheme involves the two-photon excitation of 1S-2S transitions using a linearly polarized 243-nm beam. An anisotropy is created amongst Zeeman states in 2S-4P transitions using a circularly polarized 486-nm pump beam. This anisotropy rotates the polarization of a weak, linearly polarized probe beam at 486 nm. As a result the weak probe beam "leaks" past an analyzer in the detection channel and is measured using a PMT. This signal can be related to H atom density in the probe volume. A dye laser was pumped by third harmonic of a Nd:YAG laser to create a laser beam

  8. Simultaneous electromagnetically induced transparency for two circularly polarized lasers coupled to the same linearly polarized laser in a four-level atomic system in the W scheme

    SciTech Connect

    Bahrim, Cristian; Nelson, Chris

    2011-03-15

    Electromagnetic induced transparency (EIT) can be produced in a four-level atomic system in the W scheme using a linearly polarized optical field for simultaneously slowing down two {sigma}{sup +} and {sigma}{sup -} circularly polarized optical fields. This four-level atomic system can be set up with a |{sup 1}S{sub 0}> ground state and three Zeeman levels of the |{sup 1}P{sub 1}> excited state of any alkali-metal atom placed in a weak magnetic field. We apply our W scheme to ultracold magnesium atoms for neglecting the collisional dephasing. Atomic coherences are reported after solving a density matrix master equation including radiative relaxations from Zeeman states of the |{sup 1}P{sub 1}> multiplet to the |{sup 1}S{sub 0}> ground state. The EIT feature is analyzed using the transit time between the normal dispersive region and the EIT region. The evolution of the EIT feature with the variation of the coupling field is discussed using an intuitive dressed-state representation. We analyze the sensitivity of an EIT feature to pressure broadening of the excited Zeeman states.

  9. Spin-polarized hydrogen Rydberg time-of-flight: Experimental measurement of the velocity-dependent H atom spin-polarization

    SciTech Connect

    Broderick, Bernadette M.; Lee, Yumin; Doyle, Michael B.; Chernyak, Vladimir Y.; Suits, Arthur G.; Vasyutinskii, Oleg S.

    2014-05-15

    We have developed a new experimental method allowing direct detection of the velocity dependent spin-polarization of hydrogen atoms produced in photodissociation. The technique, which is a variation on the H atom Rydberg time-of-flight method, employs a double-resonance excitation scheme and experimental geometry that yields the two coherent orientation parameters as a function of recoil speed for scattering perpendicular to the laser propagation direction. The approach, apparatus, and optical layout we employ are described here in detail and demonstrated in application to HBr and DBr photolysis at 213 nm. We also discuss the theoretical foundation for the approach, as well as the resolution and sensitivity we achieve.

  10. Insight into photofragment vector correlation by a multi-center impulsive model.

    PubMed

    Tsai, Po-Yu; Lin, King-Chuen

    2015-07-15

    A multi-center impulsive model has been recently developed to characterize the dynamic feature of product energy distribution in photodissociation of formaldehyde, H2CO → CO + H2. (J. Phys. Chem. A, 2015, 119, 29) The model is extended to predict the vector correlations among transition dipole moment μ of the parent molecule, recoil velocity v and rotational angular momentum j of the fragments produced via the transition state (TS) and roaming path. The correlation results of μ-j, j-j and μ-v vectors of the fragments are consistent with those reported using quasi-classical trajectory simulation on the global potential energy surface. In contrast to the TS route, the vector properties via the roaming path are loosely correlated. This work offers an alternative method to study stereodynamics of the photodissociation process, and is conducive to clarifying the origin of photofragment vector correlation especially for the roaming pathway. PMID:26150201

  11. A cryogenically cooled photofragment fluorescence instrument for measuring stratospheric water vapor

    NASA Technical Reports Server (NTRS)

    Weinstock, Elliot M.; Schwab, James J.; Nee, Jan Bai; Schwab, M. J.; Anderson, James G.

    1990-01-01

    An instrument developed for high-resolution daytime measurements of water vapor in the stratosphere using the technique of photofragment fluorescence is examined. A detailed description of all aspects of the instrument, as well as the results of its first two flights, are presented. The main areas of concern were optical baffling, cryogen transfer, water vapor measurement without contamination, and a dual path absorption measurement. Results of the second flight test indicate that the problems of instrument and gondola contamination, identified in the first flight test, were solved. A signal-to-noise ratio of about 50:1 for 10 sec of averaging throughout the stratosphere is achieved, as well as an altitude resolution of better than 100 m.

  12. Asymmetric branching of dissociated photofragments of HD{sup +} in an intense femtosecond laser field

    SciTech Connect

    Chatterjee, Souvik; Bhattacharyya, S. S.; Dutta, Bibhas

    2011-06-15

    We have numerically explored the asymmetry in the branching ratio of the photofragments in the photodissociation of HD{sup +} (neutral D and neutral H), leading to the possibility of localization of the electron on a chosen nucleus by careful tuning of the laser parameters. For two different frequencies we show that, starting from an initial stationary wave function, proper tuning of the pulse duration (2{sigma}) and peak intensities (I{sup 0}) of the laser pulses can lead to very different branching ratios of the two reaction channels. The results are interpreted in terms of the propagation of the nonstationary wave packet through regions having dominant radiative or nonradiative interactions at different times. We also investigate what effect the choice of initial vibrational state has on the overall asymmetry in the branching ratio of the dissociation products.

  13. Focusing a beam of ultracold spin-polarized hydrogen atoms with a helium-film-coated quasiparabolic mirror

    SciTech Connect

    Luppov, V.G. Joint Institute for Nuclear Research, Dubna ); Kaufman, W.A.; Hill, K.M.; Raymond, R.S.; Krisch, A.D. )

    1993-10-11

    We formed the first atomic-optics'' beam of electron-spin-polarized hydrogen atoms using a quasiparabolic polished copper mirror coated with a hydrogen-atom-reflecting film of superfluid [sup 4]He. The mirror was located in the gradient of an 8-T solenoidal magnetic field and mounted on an ultracold cell at 350 mK. After the focusing by the mirror surface, the beam was again focused with a sextupole magnet. The mirror, which was especially designed for operation in the magnetic field gradient of our solenoid, increased the focused beam intensity by a factor of about 7.5.

  14. Atomically-resolved mapping of polarization and electric fields across ferroelectric-oxide interfaces by Z-contrast imaging

    SciTech Connect

    Chang, Hye Jung; Kalinin, Sergei; Morozovska, A. N.; Huijben, Mark; Chu, Ying-Hao; Yu, P; Ramesh, R.; Eliseev, E. A.; Svechnikov, S. V.; Pennycook, Stephen J; Borisevich, Albina Y

    2011-01-01

    Direct atomic displacement mapping at ferroelectric interfaces by aberration corrected scanning transmission electron microscopy(STEM) (a-STEM image, b-corresponding displacement profile) is combined with Landau-Ginsburg-Devonshire theory to obtain the complete interface electrostatics in real space, including separate estimates for the polarization and intrinsic interface charge contributions.

  15. A dead-zone free ⁴He atomic magnetometer with intensity-modulated linearly polarized light and a liquid crystal polarization rotator.

    PubMed

    Wu, T; Peng, X; Lin, Z; Guo, H

    2015-10-01

    We demonstrate an all-optical (4)He atomic magnetometer experimental scheme based on an original Bell-Bloom configuration. A single intensity-modulated linearly polarized laser beam is used both for generating spin polarization within a single (4)He vapor and probing the spin precessing under a static magnetic field. The transmitted light signal from the vapor is then phase-sensitively detected at the modulation frequency and its harmonics, which lead to the atomic magnetic resonance signals. Based on this structure, a liquid crystal is added in our magnetometer system and constitutes a polarization rotator. By controlling the voltage applied on the liquid crystal, the light linear polarization vector can be kept perpendicular with the ambient magnetic field direction, which in turn provides the maximum resonance signal amplitude. Moreover, the system exhibits a magnetic-field noise floor of about 2pT/√Hz, which is not degraded due to the presence of the liquid crystal and varying magnetic field direction. The experiment results prove that our method can eliminate the dead-zone effect, improve the system spatial isotropy, and thus be suitable in mobile applications. PMID:26520938

  16. Ground state of the polar alkali-metal-atom-strontium molecules: Potential energy curve and permanent dipole moment

    SciTech Connect

    Guerout, R.; Aymar, M.; Dulieu, O.

    2010-10-15

    In this study, we investigate the structure of the polar alkali-metal-atom-strontium diatomic molecules as possible candidates for the realization of samples of ultracold polar molecular species not yet investigated experimentally. Using a quantum chemistry approach based on effective core potentials and core polarization potentials, we model these systems as effective three-valence-electron systems, allowing for calculation of electronic properties with full configuration interaction. The potential curve and the permanent dipole moment of the {sup 2}{Sigma}{sup +} ground state are determined as functions of the internuclear distance for LiSr, NaSr, KSr, RbSr, and CsSr molecules. These molecules are found to exhibit a significant permanent dipole moment, though smaller than those of the alkali-metal-atom-Rb molecules.

  17. Photoluminescence polarization anisotropy for studying long-range structural ordering within semiconductor multi-atomic alloys and organic crystals

    SciTech Connect

    Prutskij, T.; Percino, J.; Orlova, T.; Vavilova, L.

    2013-12-04

    Long-range structural ordering within multi-component semiconductor alloys and organic crystals leads to significant optical anisotropy and, in particular, to anisotropy of the photoluminescence (PL) emission. The PL emission of ternary and quaternary semiconductor alloys is polarized if there is some amount of the atomic ordering within the crystal structure. We analyze the polarization of the PL emission from the quaternary GaInAsP semiconductor alloy grown by Liquid Phase Epitaxy (LPE) and conclude that it could be caused by low degree atomic ordering within the crystal structure together with the thermal biaxial strain due to difference between the thermal expansion coefficients of the layer and the substrate. We also study the state of polarization of the PL from organic crystals in order to identify different features of the crystal PL spectrum.

  18. Measuring the spin polarization of alkali-metal atoms using nuclear magnetic resonance frequency shifts of noble gases

    SciTech Connect

    Liu, X. H.; Luo, H.; Qu, T. L. Yang, K. Y.; Ding, Z. C.

    2015-10-15

    We report a novel method of measuring the spin polarization of alkali-metal atoms by detecting the NMR frequency shifts of noble gases. We calculated the profile of {sup 87}Rb D1 line absorption cross sections. We then measured the absorption profile of the sample cell, from which we calculated the {sup 87}Rb number densities at different temperatures. Then we measured the frequency shifts resulted from the spin polarization of the {sup 87}Rb atoms and calculated its polarization degrees at different temperatures. The behavior of frequency shifts versus temperature in experiment was consistent with theoretical calculation, which may be used as compensative signal for the NMRG closed-loop control system.

  19. Development of two-color laser system for high-resolution polarization spectroscopy measurements of atomic hydrogen.

    PubMed

    Bhuiyan, A H; Satija, A; Naik, S V; Lucht, R P

    2012-09-01

    We have developed a high-spectral-resolution laser system for two-photon pump, polarization spectroscopy probe (TPP-PSP) measurements of atomic hydrogen in flames. In the TPP-PSP technique, a 243-nm laser beam excites the two-photon 1S-2S transition, and excited n=2 atoms are then detected by polarization spectroscopy of the n=2 to n=3 transition using 656-nm laser radiation. The single-frequency-mode 243 and 656-nm beams are produced using injection-seeded optical parametric generators coupled with pulsed dye amplifiers. The use of single-mode lasers allows accurate measurement of signal line shapes and intensities even with significant pulse-to-pulse fluctuations in pulse energies. Use of single-mode lasers and introduction of a scheme to select nearly constant laser energies enable repeatable extraction of important spectral features in atomic hydrogen transitions. PMID:22940950

  20. Strong-field atomic ionization in an elliptically polarized laser field and a constant magnetic field

    NASA Astrophysics Data System (ADS)

    Rylyuk, V. M.

    2016-05-01

    Within the framework of the quasistationary quasienergy state (QQES) formalism, the tunneling and multiphoton ionization of atoms and ions subjected to a perturbation by a high intense laser radiation field of an arbitrary polarization and a constant magnetic field are considered. On the basis of the exact solution of the Schrödinger equation and the Green's function for the electron moving in an arbitrary laser field and crossed constant electric and magnetic fields, the integral equation for the complex quasienergy and the energy spectrum of the ejected electron are derived. Using the "imaginary-time" method, the extremal subbarrier trajectory of the photoelectron moving in a nonstationary laser field and a constant magnetic field are considered. Within the framework of the QQES formalism and the quasiclassical perturbation theory, ionization rates when the Coulomb interaction of the photoelectron with the parent ion is taken into account at arbitrary values of the Keldysh parameter are derived. The high accuracy of rates is confirmed by comparison with the results of numerical calculations. Simple analytical expressions for the ionization rate with the Coulomb correction in the tunneling and multiphoton regimes in the case of an elliptically polarized laser beam propagating at an arbitrary angle to the constant magnetic field are derived and discussed. The limits of small and large magnetic fields and low and high frequency of a laser field are considered in details. It is shown that in the presence of a nonstationary laser field perturbation, the constant magnetic field may either decrease or increase the ionization rate. The analytical consideration and numerical calculations also showed that the difference between the ionization rates for an s electron in the case of right- and left-elliptically polarized laser fields is especially significant in the multiphoton regime for not-too-high magnetic fields and decreases as the magnetic field increases. The paper

  1. Energetic neutral atom imaging with the Polar CEPPAD/IPS instrument: Initial forward modeling results

    SciTech Connect

    Henderson, M.G.; Reeves, G.D.; Moore, K.R.; Spence, H.E.; Jorgensen, A.M.; Fennell, J.F.; Blake, J.B.; Roelof, E.C.

    1997-12-31

    Although the primary function of the CEP-PAD/IPS instrument on Polar is the measurement of energetic ions in-situ, it has also proven to be a very capable Energetic neutral Atom (ENA) imager. Raw ENA images are currently being constructed on a routine basis with a temporal resolution of minutes during both active and quiet times. However, while analyses of these images by themselves provide much information on the spatial distribution and dynamics of the energetic ion population in the ring current, detailed modeling is required to extract the actual ion distributions. In this paper, the authors present the initial results of forward modeling an IPS ENA image obtained during a small geo-magnetic storm on June 9, 1997. The equatorial ion distribution inferred with this technique reproduces the expected large noon/midnight and dawn/dusk asymmetries. The limitations of the model are discussed and a number of modifications to the basic forward modeling technique are proposed which should significantly improve its performance in future studies.

  2. Energetic Neutral Atom Imaging with the POLAR CEPPAD/ IPS Instrument : Initial Forward Modeling Results

    NASA Technical Reports Server (NTRS)

    Henderson, M. G.; Reeves, G. D.; Moore, K. R.; Spence, H. E.; Jorgensen, A. M.; Fennell, J. F.; Blake, J. B.; Roelof, E. C.

    1999-01-01

    Although the primary function of the CEPPAD/IPS instrument on Polar is the measurement of energetic ions in-situ, it has also proven to be a very capable Energetic Neutral Atom (ENA) imager. Raw ENA images are currently being constructed on a routine basis with a temporal resolution of minutes during both active and quiet times. However, while analyses of these images by themselves provide much information on the spatial distribution and dynamics of the energetic ion population in the ring current. detailed modeling is required to extract the actual ion distributions. In this paper. we present the initial results of forward modeling an IPS ENA image obtained during a small geo-magnetic storm on June 9, 1997. The equatorial ion distribution inferred with this technique reproduces the expected large noon/midnight and dawn/dusk asymmetries. The limitations of the model are discussed and a number of modifications to the basic forward modeling technique are proposed which should significantly improve its performance in future studies.

  3. Polarization squeezing of light by single passage through an atomic vapor

    NASA Astrophysics Data System (ADS)

    Barreiro, S.; Valente, P.; Failache, H.; Lezama, A.

    2011-09-01

    We have studied relative-intensity fluctuations for a variable set of orthogonal elliptic polarization components of a linearly polarized laser beam traversing a resonant 87Rb vapor cell. Significant polarization squeezing at the threshold level (-3dB) required for the implementation of several continuous-variable quantum protocols was observed. The extreme simplicity of the setup, which is based on standard polarization components, makes it particularly convenient for quantum information applications.

  4. Predictions of laser-cooling temperatures for multilevel atoms in three-dimensional polarization-gradient fields

    SciTech Connect

    Dunn, Josh W.; Greene, Chris H.

    2006-03-15

    We analyze the dynamics of atom-laser interactions for atoms having multiple, closely spaced, excited-state hyperfine manifolds. The system is treated fully quantum mechanically, including the atom's center-of-mass degree of freedom, and motion is described in a polarization gradient field created by a three-dimensional laser configuration. We develop the master equation describing this system, and then specialize it to the low-intensity limit by adiabatically eliminating the excited states. We show how this master equation can be simulated using the Monte Carlo wave function technique, and we provide details on the implementation of this procedure. Monte Carlo calculations of steady state atomic momentum distributions for two fermionic alkaline earth isotopes, {sup 25}Mg and {sup 87}Sr, interacting with a three-dimensional lin-perpendicular-lin laser configuration are presented, providing estimates of experimentally achievable laser-cooling temperatures.

  5. Probing Membrane Order and Topography in Supported Lipid Bilayers by Combined Polarized Total Internal Reflection Fluorescence-Atomic Force Microscopy

    PubMed Central

    Oreopoulos, John; Yip, Christopher M.

    2009-01-01

    Determining the local structure, dynamics, and conformational requirements for protein-protein and protein-lipid interactions in membranes is critical to understanding biological processes ranging from signaling to the translocating and membranolytic action of antimicrobial peptides. We report here the application of a combined polarized total internal reflection fluorescence microscopy-in situ atomic force microscopy platform. This platform's ability to image membrane orientational order was demonstrated on DOPC/DSPC/cholesterol model membranes containing the fluorescent membrane probe, DiI-C20 or BODIPY-PC. Spatially resolved order parameters and fluorophore tilt angles extracted from the polarized total internal reflection fluorescence microscopy images were in good agreement with the topographical details resolved by in situ atomic force microscopy, portending use of this technique for high-resolution characterization of membrane domain structures and peptide-membrane interactions. PMID:19254557

  6. VARIATIONS IN THE HELIOSPHERIC POLAR ENERGETIC NEUTRAL ATOM FLUX OBSERVED BY THE INTERSTELLAR BOUNDARY EXPLORER

    SciTech Connect

    Reisenfeld, D. B.; Janzen, P. H.; Allegrini, F.; McComas, D. J. E-mail: paul.janzen@umontana.edu E-mail: dmccomas@swri.org; and others

    2012-03-10

    The ecliptic poles are observed continuously by the Interstellar Boundary Explorer (IBEX); thus, it is possible to discern temporal variations in the energetic neutral atoms (ENAs) from the outer heliosphere on timescales much shorter than the time it takes for IBEX to generate a full sky map (six months). Observations indicate that the ENA flux from the polar directions incident at Earth has been steadily decreasing for the two-year period from 2008 December through 2011 February. Over the IBEX-Hi energy range, the decrease in flux is energy dependent, varying at the south ecliptic pole from no drop at 0.71 keV, to 70% at 1.1 keV. At higher energies the drop ranges between 10% and 50%. The decline observed at the north ecliptic pole is as high as 48%, also at 1.1 keV. The trend correlates with the steady decline in solar wind dynamic pressure observed at 1 AU between 2005 and 2009, the likely period when solar wind protons that provide the source for ENAs observed by IBEX would have been outbound from the Sun. We propose a method by which the correlation between the 1 AU solar wind dynamic pressure and the ENA-derived pressure within the inner heliosheath (IHS) can be used to estimate the distance to the termination shock and the thickness of the IHS in the direction of the ecliptic poles. Our new analysis based on IBEX data shows the TS distances to be 110 AU and 134 AU at the south and north poles, respectively, and the corresponding IHS thicknesses to be 55 AU and 82 AU. Our analysis is consistent with the notion that the observed ENA fluxes originate in the IHS and their variations are driven by the solar wind as it evolves through the solar cycle.

  7. Scattering of polarized laser light by an atomic gas in free space: A quantum stochastic differential equation approach

    SciTech Connect

    Bouten, Luc; Stockton, John; Sarma, Gopal; Mabuchi, Hideo

    2007-05-15

    We propose a model, based on a quantum stochastic differential equation (QSDE), to describe the scattering of polarized laser light by an atomic gas. The gauge terms in the QSDE account for the direct scattering of the laser light into different field channels. Once the model has been set, we can rigorously derive quantum filtering equations for balanced polarimetry and homodyne detection experiments, study the statistics of output processes, and investigate a strong driving, weak coupling limit.

  8. Photoelectron-photofragment coincidence spectroscopy in a cryogenically cooled linear electrostatic ion beam trap

    SciTech Connect

    Johnson, Christopher J.; Shen, Ben B.; Poad, Berwyck L. J.; Continetti, Robert E.

    2011-10-15

    A cryogenically cooled linear electrostatic ion beam trap for use in photoelectron-photofragment coincidence (PPC) spectroscopy is described. Using this instrument, anions created in cold, low-duty-cycle sources can be stored for many seconds in a {approx}20 K environment to cool radiatively, removing energetic uncertainties due to vibrationally excited precursor anions. This apparatus maintains a well-collimated beam necessary for high-resolution fragment imaging and the high experimental duty cycle needed for coincidence experiments. Ion oscillation is bunched and phase-locked to a modelocked laser, ensuring temporal overlap between ion bunches and laser pulses and that ions are intersected by the laser only when travelling in one direction. An electron detector is housed in the field-free center of the trap, allowing PPC experiments to be carried out on ions while they are stored and permitting efficient detection of 3-dimensional electron and neutral recoil trajectories. The effects of trapping parameters on the center-of-mass trajectories in the laser-ion interaction region are explored to optimize neutral particle resolution, and the impact of bunching on ion oscillation is established. Finally, an initial demonstration of radiative cooling is presented.

  9. Pyrenyl Derivative with a Four-Atom Linker That Can Probe the Local Polarity of Pyrene-Labeled Macromolecules.

    PubMed

    Farhangi, Shiva; Duhamel, Jean

    2016-02-01

    The fluorescent probe 1-pyrenemethoxyethanol (PyMeEGOH) was designed to replace commercially available 1-pyrenebutanol (PyButOH) as an alternative fluorescent label to probe the internal dynamics and interior polarity of macromolecules by steady-state and time-resolved fluorescence. While excimer formation and sensitivity to solvent polarity are two well-recognized properties of pyrene, much less known is that these properties are often mutually exclusive when a 1-pyrenebutyl derivative is used to prepare pyrene-labeled macromolecules (PyLMs). As the sensitivity of pyrene to solvent polarity is a result of its symmetry, attaching a butyl group to pyrene breaks the symmetry of pyrene, so that the 1-pyrenebutyl derivatives are much less sensitive to the polarity of their environment compared to unmodified pyrene. This report demonstrates that replacement of a methylene group in the β-position of PyButOH by an oxygen atom, such as in PyMeEGOH, restores the sensitivity of this pyrene derivative to the polarity of its local environment to the same level as that of molecular pyrene without impeding pyrene excimer formation upon incorporation into PyLMs. PMID:26734846

  10. Atomic and electronic structure of polar Fe2O3(0001)/MgO(111) interfaces

    NASA Astrophysics Data System (ADS)

    Pande, K.; Gajdardziska-Josifovska, M.; Weinert, M.

    2012-07-01

    We present a first-principles investigation of the structural, electronic, and magnetic properties of ultrathin Fe2O3(0001) films on a polar MgO(111) substrate. The results imply that the heterointerface is atomically abrupt with oxidelike stacking for film thicknesses between ˜1.5 and 8.5 Å. The Fe-Fe bilayer (nominal separation of 0.59 Å in Fe2O3) at the interface collapses into an “Fe2” monolayer. Both electronic polarization and structural relaxations effectively screen the dipole field of the polar interface system. The structural relaxations—consisting of interpenetration, separation, and merger of Fe and oxygen planes—are particularly drastic in the three- and four-bilayers-thick films, giving rise to barrierless movement of oxygen towards the surface and the formation of an “Fe2|FeO3” layer structure not seen in hematite. Comparisons to calculations of unsupported polar Fe2O3(0001) slabs demonstrate that these unusual changes in stacking sequence and electronic structure are associated with the polar nature of this oxide heterointerface.

  11. Polarized internal target apparatus

    DOEpatents

    Holt, R.J.

    1984-10-10

    A polarized internal target apparatus with a polarized gas target of improved polarization and density (achieved by mixing target gas atoms with a small amount of alkali metal gas atoms, and passing a high intensity polarized light source into the mixture to cause the alkali metal gas atoms to become polarized which interact in spin exchange collisions with target gas atoms yielding polarized target gas atoms) is described.

  12. Polarized internal target apparatus

    DOEpatents

    Holt, Roy J.

    1986-01-01

    A polarized internal target apparatus with a polarized gas target of improved polarization and density achieved by mixing target gas atoms with a small amount of alkali metal gas atoms, and passing a high intensity polarized light source into the mixture to cause the alkali metal gas atoms to become polarized which interact in spin exchange collisions with target gas atoms yielding polarized target gas atoms.

  13. Doping, adsorption, and polarity of atomic-layer materials: A predictive theory from systematic first-principles study

    NASA Astrophysics Data System (ADS)

    Saito, Susumu; Fujimoto, Yoshitaka; Koretsune, Takashi

    2015-03-01

    Based on the extensive first-principles electronic-structure study of various doped hexagonal boron-nitride (h-BN) atomic layers as well as that of various doped graphene and carbon nanotubes, we propose a simple but predictive theory of polarity in doped atomic-layer materials. We first report the electronic structure of the pristine h-BN, h-BN layers with B and B3N vacancies which have been experimentally produced and observed frequently, and doped h-BN layers, and show that both p-type and n-type h-BN layers can be produced in a variety of ways. We next review the electronic structure of doped graphene and carbon nanotubes and the effect of the H adsorption which can even change the polarity of the system. Finally we propose a simple but predictive theory which is based on the number of valence electrons of each system, and can explain the polarities of all the h-BN, graphene, and nanotube-based systems studied so far. Supported by MEXT 25107005 and 25104711, JSPS 22740252 and 26390062, and MEST TIES project.

  14. Implementation of Outstanding Electronic Transport in Polar Covalent Boron Nitride Atomic Chains: another Extraordinary Odd-Even Behaviour

    PubMed Central

    Xu, Xiaodong; Li, Weiqi; Liu, Linhua; Feng, Jikang; Jiang, Yongyuan; Tian, Wei Quan

    2016-01-01

    A theoretical investigation of the unique electronic transport properties of the junctions composed of boron nitride atomic chains bridging symmetric graphene electrodes with point-contacts is executed through non-equilibrium Green’s function technique in combination with density functional theory. Compared with carbon atomic chains, the boron nitride atomic chains have an alternative arrangement of polar covalent B-N bonds and different contacts coupling electrodes, showing some unusual properties in functional atomic electronic devices. Remarkably, they have an extraordinary odd-even behavior of conductivity with the length increase. The rectification character and negative differential resistance of nonlinear current-voltage characteristics can be achieved by manipulating the type of contacts between boron nitride atomic chains bridges and electrodes. The junctions with asymmetric contacts have an intrinsic rectification, caused by stronger coupling in the C-N contact than the C-B contact. On the other hand, for symmetric contact junctions, it is confirmed that the transport properties of the junctions primarily depend on the nature of contacts. The junctions with symmetric C-N contacts have higher conductivity than their C-B contacts counterparts. Furthermore, the negative differential resistances of the junctions with only C-N contacts is very conspicuous and can be achieved at lower bias. PMID:27211110

  15. Implementation of Outstanding Electronic Transport in Polar Covalent Boron Nitride Atomic Chains: another Extraordinary Odd-Even Behaviour.

    PubMed

    Xu, Xiaodong; Li, Weiqi; Liu, Linhua; Feng, Jikang; Jiang, Yongyuan; Tian, Wei Quan

    2016-01-01

    A theoretical investigation of the unique electronic transport properties of the junctions composed of boron nitride atomic chains bridging symmetric graphene electrodes with point-contacts is executed through non-equilibrium Green's function technique in combination with density functional theory. Compared with carbon atomic chains, the boron nitride atomic chains have an alternative arrangement of polar covalent B-N bonds and different contacts coupling electrodes, showing some unusual properties in functional atomic electronic devices. Remarkably, they have an extraordinary odd-even behavior of conductivity with the length increase. The rectification character and negative differential resistance of nonlinear current-voltage characteristics can be achieved by manipulating the type of contacts between boron nitride atomic chains bridges and electrodes. The junctions with asymmetric contacts have an intrinsic rectification, caused by stronger coupling in the C-N contact than the C-B contact. On the other hand, for symmetric contact junctions, it is confirmed that the transport properties of the junctions primarily depend on the nature of contacts. The junctions with symmetric C-N contacts have higher conductivity than their C-B contacts counterparts. Furthermore, the negative differential resistances of the junctions with only C-N contacts is very conspicuous and can be achieved at lower bias. PMID:27211110

  16. Implementation of Outstanding Electronic Transport in Polar Covalent Boron Nitride Atomic Chains: another Extraordinary Odd-Even Behaviour

    NASA Astrophysics Data System (ADS)

    Xu, Xiaodong; Li, Weiqi; Liu, Linhua; Feng, Jikang; Jiang, Yongyuan; Tian, Wei Quan

    2016-05-01

    A theoretical investigation of the unique electronic transport properties of the junctions composed of boron nitride atomic chains bridging symmetric graphene electrodes with point-contacts is executed through non-equilibrium Green’s function technique in combination with density functional theory. Compared with carbon atomic chains, the boron nitride atomic chains have an alternative arrangement of polar covalent B-N bonds and different contacts coupling electrodes, showing some unusual properties in functional atomic electronic devices. Remarkably, they have an extraordinary odd-even behavior of conductivity with the length increase. The rectification character and negative differential resistance of nonlinear current-voltage characteristics can be achieved by manipulating the type of contacts between boron nitride atomic chains bridges and electrodes. The junctions with asymmetric contacts have an intrinsic rectification, caused by stronger coupling in the C-N contact than the C-B contact. On the other hand, for symmetric contact junctions, it is confirmed that the transport properties of the junctions primarily depend on the nature of contacts. The junctions with symmetric C-N contacts have higher conductivity than their C-B contacts counterparts. Furthermore, the negative differential resistances of the junctions with only C-N contacts is very conspicuous and can be achieved at lower bias.

  17. Roles of Atomic Injection Rate and External Magnetic Field on Optical Properties of Elliptical Polarized Probe Light

    NASA Astrophysics Data System (ADS)

    Karimi, R.; Asadpour, S. H.; Batebi, S.; Rahimpour Soleimani, H.

    2016-01-01

    In this paper we investigate the optical properties of an open four-level tripod atomic system driven by an elliptically polarized probe field in the presence of the external magnetic field and compare its properties with the corresponding closed system. Our result reveals that absorption, dispersion and group velocity of probe field can be manipulated by adjusting the phase difference between the two circularly polarized components of a single coherent field, magnetic field and cavity parameters i.e. the atomic exit rate from cavity and atomic injection rates. We show that the system can exhibit multiple electromagnetically induced transparency windows in the presence of the external magnetic field. The numerical result shows that the probe field in the open system can be amplified by appropriate choice of cavity parameters, while in the closed system with introduce appropriate phase difference between fields the probe field can be enhanced. Also it is shown that the group velocity of light pulse can be controlled by external magnetic field, relative phase of applied fields and cavity parameters. By changing the parameters the group velocity of light pulse changes from subluminal to superluminal light propagation and vice versa.

  18. Magneto-optical polarization rotation in a ladder-type atomic system for tunable offset locking

    NASA Astrophysics Data System (ADS)

    Parniak, Michał; Leszczyński, Adam; Wasilewski, Wojciech

    2016-04-01

    We demonstrate an easily tunable locking scheme for stabilizing frequency-sum of two lasers on a two-photon ladder transition based on polarization rotation in warm rubidium vapors induced by magnetic field and circularly polarized drive field. Unprecedented tunability of the two-photon offset frequency is due to strong splitting and shifting of magnetic states in external field. In our experimental setup, we achieve two-photon detuning of up to 700 MHz.

  19. QED radiative corrections and many-body effects in atoms: vacuum polarization and binding energy shifts in alkali metals

    NASA Astrophysics Data System (ADS)

    Ginges, J. S. M.; Berengut, J. C.

    2016-05-01

    We calculate vacuum polarization corrections to the binding energies in neutral alkali atoms Na through to the superheavy element E119. We employ the relativistic Hartree–Fock method to demonstrate the importance of relaxation of the electronic core and the correlation potential method to study the effects of second and higher orders of perturbation theory. These many-body effects are sizeable for all orbitals, though particularly important for orbitals with angular momentum quantum number l\\gt 0. The orders of magnitude enhancement for d waves produces shifts that, for Rb and the heavier elements, are larger than those for p waves and only an order of magnitude smaller than the s-wave shifts. The many-body enhancement mechanisms that operate for vacuum polarization apply also to the larger self-energy corrections.

  20. Coherent manipulation of a single magnetic atom using polarized single electron transport in a double quantum dot

    NASA Astrophysics Data System (ADS)

    Lai, Wenxi; Yang, Wen

    2015-10-01

    We consider theoretically a magnetic impurity spin driven by polarized electrons tunneling through a double-quantum-dot system. The spin-blockade effect and spin conservation in the system make the magnetic impurity sufficiently interact with each transferring electron. As a result, a single collected electron carries information about spin change of the magnetic impurity. The scheme may develop all-electrical manipulation of magnetic atoms by means of single electrons, which is significant for the implementation of scalable logical gates in information processing systems.

  1. Control of threshold enhancements in harmonic generation by atoms in a two-color laser field with orthogonal polarizations

    NASA Astrophysics Data System (ADS)

    Frolov, M. V.; Manakov, N. L.; Sarantseva, T. S.; Silaev, A. A.; Vvedenskii, N. V.; Starace, Anthony F.

    2016-02-01

    Threshold phenomena (or channel-closing effects) are analyzed in high-order harmonic generation (HHG) by atoms in a two-color laser field with orthogonal linearly polarized components of a fundamental field and its second harmonic. We show that the threshold behavior of HHG rates for the case of a weak second harmonic component is sensitive to the parity of a closing multiphoton ionization channel and the spatial symmetry of the initial bound state of the target atom, while for the case of comparable intensities of both components, suppression of threshold phenomena is observed as the relative phase between the components of a two-color field varies. A quantum orbit analysis as well as phenomenological considerations in terms of Baz' theory of threshold phenomena [Zh. Eksp. Teor. Fiz. 33, 923 (1957)] are presented in order to describe and explain the major features of threshold phenomena in HHG by a two-color field.

  2. Fast automated placement of polar hydrogen atoms in protein-ligand complexes

    PubMed Central

    2009-01-01

    Background Hydrogen bonds play a major role in the stabilization of protein-ligand complexes. The ability of a functional group to form them depends on the position of its hydrogen atoms. An accurate knowledge of the positions of hydrogen atoms in proteins is therefore important to correctly identify hydrogen bonds and their properties. The high mobility of hydrogen atoms introduces several degrees of freedom: Tautomeric states, where a hydrogen atom alters its binding partner, torsional changes where the position of the hydrogen atom is rotated around the last heavy-atom bond in a residue, and protonation states, where the number of hydrogen atoms at a functional group may change. Also, side-chain flips in glutamine and asparagine and histidine residues, which are common crystallographic ambiguities must be identified before structure-based calculations can be conducted. Results We have implemented a method to determine the most probable hydrogen atom positions in a given protein-ligand complex. Optimality of hydrogen bond geometries is determined by an empirical scoring function which is used in molecular docking. This allows to evaluate protein-ligand interactions with an established model. Also, our method allows to resolve common crystallographic ambiguities such as as flipped amide groups and histidine residues. To ensure high speed, we make use of a dynamic programming approach. Conclusion Our results were checked against selected high-resolution structures from an external dataset, for which the positions of the hydrogen atoms have been validated manually. The quality of our results is comparable to that of other programs, with the advantage of being fast enough to be applied on-the-fly for interactive usage or during score evaluation. PMID:20298519

  3. [The Measuring Method of Atomic Polarization of Alkali Metal Vapor Based on Optical Rotation and the Analysis of the Influence Factors].

    PubMed

    Shang, Hui-ning; Quan, Wei; Chen, Yao; Li, Yang; Li, Hong

    2016-02-01

    High sensitivity measurements of inertia and magnetic field could be achieved by utilizing a category of devices, which manipulate the atomic spins in the spin-exchange-relaxation-free regime. The alkali cell which contains the alkali metal vapor is used to sense magnetic field and inertia. The atomic number density of alkali vapor and the polarization of alkali metal vapor are two of the most important parameters of the cell. They play an important role in the research on atomic spins in the spin-exchange-relaxation-free regime. Besides, optical polarization plays an important role in quantum computing and atomic physics. We propose a measurement of alkali vapor polarization and alkali number density by detecting the optical rotation in one system. This method simplifies existing experimental equipment and processes. A constant bias magnetic field is applied and the Faraday rotation angle is detected by a bunch of the probe beam to deduce alkali-metal density. Then the magnetic field is closed and a bunch of the pump laser is utilized to polarize alkali-metal. Again, the probe beam is utilized to obtain the polarization of alkali metal. The alkali density obtained at first is used to deduce the polarization. This paper applies a numerical method to analyze the Faraday rotation and the polarization rotation. According to the numerical method, the optimal wavelength for the experiment is given. Finally, the fluctuation of magnetic field and wavelength on signal analysis are analyzed. PMID:27209720

  4. Alkali-metal-atom polarization imaging in high-pressure optical-pumping cells

    NASA Astrophysics Data System (ADS)

    Baranga, A. Ben-Amar; Appelt, S.; Erickson, C. J.; Young, A. R.; Happer, W.

    1998-09-01

    We present a detailed experimental analysis of Rb-polarization imaging in high-pressure gas cells. The Rb vapor in these cells is optically pumped by high-power diode-laser arrays. We present images for high (35 G) and low (4 G) magnetic fields and for different He and Xe buffer-gas mixtures. We demonstrate that high-field imaging provides an absolute measurement of the Rb-polarization distribution in the cell, based on the fact that a spin-temperature distribution of the hyperfine magnetic sublevels is established in high-pressure buffer gases. A survey of various mechanisms that broaden the Rb magnetic-resonance lines is presented. These broadening mechanisms determine the limits of the spatial resolution achievable for images of the Rb-polarization distribution.

  5. Vector correlations in photodissociation of polarized polyatomic molecules beyond the axial recoil limit.

    PubMed

    Krasilnikov, Mikhail B; Kuznetsov, Vladislav V; Suits, Arthur G; Vasyutinskii, Oleg S

    2011-05-14

    We present the full quantum mechanical theory of the angular momentum distributions of photofragments produced in photolysis of oriented/aligned parent polyatomic molecules beyond the axial recoil limit. This paper generalizes the results of Underwood and Powis(28,29) to the case of non-axial recoil photodissociation of an arbitrary polyatomic molecule. The spherical tensor approach is used throughout this paper. We show that the recoil angular distribution of the angular momentum polarization of each of the photofragments can be presented in a universal spherical tensor form valid for photolysis in diatomic or polyatomic molecules, irrespective of the reaction mechanism. The angular distribution can be written as an expansion over the Wigner D-functions in terms of the set of the anisotropy-transforming coefficients c(K(i)q(i))(K) (k(d), K(0)) which contain all of the information about the photodissociation dynamics and can be either determined from experiment, or computed from quantum mechanical theory. An important new conservation rule is revealed through the analysis, namely that the component q(i) of the initial reagent polarization rank K(i) and the photofragment polarization rank K onto the photofragment recoil direction k is preserved in any photolysis reaction. Both laboratory and body frame expressions for the recoil angle dependence of the photofragment angular momentum polarization are presented. The parent molecule polarization is shown to lead to new terms in the obtained photofragment angular distributions compared with the isotropic case. In particular, the terms with |q(i)| > 2 can appear which are shown to manifest angular momentum helicity non-conservation in the reaction. The expressions for the coefficients c(K(i)q(i))(K) (k(d), K(0)) have been simplified using the quasiclassical approximation in the high-J limit which allows for introducing the dynamical functions and the rotation factors which describe the decreasing of the photofragment

  6. Polarization of Lyman-(alpha) Radiation from Atomic Hydrogen Excited by Electron Impact from Near-Threshold to 1800eV

    NASA Technical Reports Server (NTRS)

    James, G. K.; Slevin, J. A.; Dziczek, D.

    1996-01-01

    The polarization of Lyman-(alpha) radiation, produced by electron impact excitation of atomic hydrogen, has been measured for the first time over the extended energy range from near-threshold to 1800eV. Measurements were obtained in a crossed-beams experiment using a silica-reflection linear polarization analyzer in tandem with a vacuum ultraviolet (VUV) monochromator to isolate the emitted line radiation.

  7. Bibenzyl- and stilbene-core compounds with non-polar linker atom substituents as selective ligands for estrogen receptor beta.

    PubMed

    Waibel, Michael; De Angelis, Meri; Stossi, Fabio; Kieser, Karen J; Carlson, Kathryn E; Katzenellenbogen, Benita S; Katzenellenbogen, John A

    2009-09-01

    A series of structurally simple bibenzyl-diol and stilbene-diol core molecules, structural analogs of the well-known hexestrol and diethylstilbestrol non-steroidal estrogens, were prepared and evaluated as estrogen receptor (ER) subtype-selective ligands. Analysis of their ERalpha and ERbeta binding showed that certain substitution patterns engendered binding affinities that were >100-fold selective for ERbeta. When further investigated in cell-based gene transcription assays, some molecules showed similarly high relative transcriptional potency selectivity in favor of ERbeta. Interestingly, the most ERbeta-selective molecules were those bearing non-polar substituents on one of the internal carbon atoms. These compounds should be useful probes for determining the physiological roles of ERbeta, and they might lead to the development of more selective and thus safer pharmaceuticals. PMID:19286283

  8. Quantum Drude oscillator model of atoms and molecules: Many-body polarization and dispersion interactions for atomistic simulation

    NASA Astrophysics Data System (ADS)

    Jones, Andrew P.; Crain, Jason; Sokhan, Vlad P.; Whitfield, Troy W.; Martyna, Glenn J.

    2013-04-01

    Treating both many-body polarization and dispersion interactions is now recognized as a key element in achieving the level of atomistic modeling required to reveal novel physics in complex systems. The quantum Drude oscillator (QDO), a Gaussian-based, coarse grained electronic structure model, captures both many-body polarization and dispersion and has linear scale computational complexity with system size, hence it is a leading candidate next-generation simulation method. Here, we investigate the extent to which the QDO treatment reproduces the desired long-range atomic and molecular properties. We present closed form expressions for leading order polarizabilities and dispersion coefficients and derive invariant (parameter-free) scaling relationships among multipole polarizability and many-body dispersion coefficients that arise due to the Gaussian nature of the model. We show that these “combining rules” hold to within a few percent for noble gas atoms, alkali metals, and simple (first-row hydride) molecules such as water; this is consistent with the surprising success that models with underlying Gaussian statistics often exhibit in physics. We present a diagrammatic Jastrow-type perturbation theory tailored to the QDO model that serves to illustrate the rich types of responses that the QDO approach engenders. QDO models for neon, argon, krypton, and xenon, designed to reproduce gas phase properties, are constructed and their condensed phase properties explored via linear scale diffusion Monte Carlo (DMC) and path integral molecular dynamics (PIMD) simulations. Good agreement with experimental data for structure, cohesive energy, and bulk modulus is found, demonstrating a degree of transferability that cannot be achieved using current empirical models or fully ab initio descriptions.

  9. Polarization spectroscopy and laser-locking for excitation of ultracold potassium atoms

    NASA Astrophysics Data System (ADS)

    Conover, Charles; Eberhart, Max; Adamson, Philip

    2016-05-01

    We report on the use of polarization spectroscopy to lock the frequency of an external-cavity diode laser to a the 4s - 4 p1/2 (770 nm), 4s - 4 p3/2 (767 nm) and 4s - 5 p1/2 and 4s - 5 p3/2 (405 nm) transitions in potassium. A rate equation model is in good agreement with the observed lineshapes and the D2 transition lineshapes agree with prior experiments. We have used the dispersion shaped lines to lock the frequency of lasers for probing a magneto-optical trap's density on the D1 line and for stepwise excitation of potassium Rydberg states using the 4s - 5 p3/2 transition. The technique has proven particularly helpful by enabling modulation-free locking of blue diode lasers. This research was supported by the National Science Foundation under Grant PHY-1126599.

  10. Unravelling the role of quantum interference in the weak-field laser phase modulation control of photofragment distributions.

    PubMed

    García-Vela, Alberto; Henriksen, Niels E

    2016-02-14

    The role played by quantum interference in the laser phase modulation coherent control of photofragment distributions in the weak-field regime is investigated in detail in this work. The specific application involves realistic wave packet calculations of the transient vibrational populations of the Br2(B,vf) fragment produced upon predissociation of the Ne-Br2(B) complex, which is excited to a superposition of overlapping resonance states using different fixed bandwidth pulses where the linear chirps are varied. The postpulse transient phase modulation effects observed on fragment populations for a long time window are explained in terms of the mechanism of interference between overlapping resonances. A detailed description of how the interference mechanism affects the magnitude and the time window of the phase control effects is also provided. In the light of the results, the conditions to maximize phase modulation control on fragment distributions are discussed. PMID:26799495

  11. Universal ultracold collision rates for polar molecules of two alkali-metal atoms

    NASA Astrophysics Data System (ADS)

    Julienne, Paul; Hanna, Thomas; Idziaszek, Zbigniew

    2011-05-01

    Highly reactive ultracold polar molecules have universal near-threshold reaction rate constants that depend only on the long-range interaction potential, as shown for the KRb molecule. We extend these calculations to estimate universal reaction rate constants for the bosonic and fermionic isotopes of the reactive species LiNa, LiK, LiRb, LiCs, and also the universal vibrational quenching rate constants for vibrationally excited states of the non-reactive species NaK, NaRb, NaCs, KCs, and RbCs. We also examine the variation with electric field of the universal collision rates for these species in quasi-2D geometry in a one-dimensional optical lattice. For many of these species an electric field of a few kV/cm perpendicular to the lattice plane should be effective in shielding the molecules from destructive collisions even at relatively modest lattice confinement strength. Supported by an AFOSR MURI and a Polish government grant.

  12. Polarization control of an infrared silicon light-emitting diode by dressed photons and analyses of the spatial distribution of doped boron atoms

    NASA Astrophysics Data System (ADS)

    Kawazoe, Tadashi; Nishioka, Katsuhiro; Ohtsu, Motoichi

    2015-12-01

    This paper reports the fabrication of a polarization-controlled infrared LED fabricated by dressed-photon-phonon (DPP)-assisted annealing of a bulk Si crystal. For the DPP-assisted annealing, linearly polarized infrared light with a wavelength of 1.342 μm was made normally incident on the top surface of the crystal. The photon energy at the peak of the emitted light spectrum of the fabricated LED was close to that of the light irradiated during the DPP-assisted annealing. A degree of polarization of as large as 0.07 was obtained. The spatial distribution of the doped B atoms in the fabricated LED was measured, and the following findings were obtained: (1) B atoms formed pairs in which the separation between the two B atoms was three times the lattice constant of the Si crystal; and (2) the B atom pairs were apt to orient along the direction perpendicular to the propagation direction and to the polarization direction of the light irradiated during the DPP-assisted annealing. Based on these findings (1) and (2), photon breeding was confirmed with respect to photon energy and spin, respectively.

  13. High-speed atomic force microscopy reveals strongly polarized movement of clostridial collagenase along collagen fibrils.

    PubMed

    Watanabe-Nakayama, Takahiro; Itami, Masahiro; Kodera, Noriyuki; Ando, Toshio; Konno, Hiroki

    2016-01-01

    Bacterial collagenases involved in donor infection are widely applied in many fields due to their high activity and specificity; however, little is known regarding the mechanisms by which bacterial collagenases degrade insoluble collagen in host tissues. Using high-speed atomic force microscopy, we simultaneously visualized the hierarchical structure of collagen fibrils and the movement of a representative bacterial collagenase, Clostridium histolyticum type I collagenase (ColG), to determine the relationship between collagen structure and collagenase movement. Notably, ColG moved ~14.5 nm toward the collagen N terminus in ~3.8 s in a manner dependent on a catalytic zinc ion. While ColG was engaged, collagen molecules were not only degraded but also occasionally rearranged to thicken neighboring collagen fibrils. Importantly, we found a similarity of relationship between the enzyme-substrate interface structure and enzyme migration in collagen-collagenase and DNA-nuclease systems, which share a helical substrate structure, suggesting a common strategy in enzyme evolution. PMID:27373458

  14. High-speed atomic force microscopy reveals strongly polarized movement of clostridial collagenase along collagen fibrils

    PubMed Central

    Watanabe-Nakayama, Takahiro; Itami, Masahiro; Kodera, Noriyuki; Ando, Toshio; Konno, Hiroki

    2016-01-01

    Bacterial collagenases involved in donor infection are widely applied in many fields due to their high activity and specificity; however, little is known regarding the mechanisms by which bacterial collagenases degrade insoluble collagen in host tissues. Using high-speed atomic force microscopy, we simultaneously visualized the hierarchical structure of collagen fibrils and the movement of a representative bacterial collagenase, Clostridium histolyticum type I collagenase (ColG), to determine the relationship between collagen structure and collagenase movement. Notably, ColG moved ~14.5 nm toward the collagen N terminus in ~3.8 s in a manner dependent on a catalytic zinc ion. While ColG was engaged, collagen molecules were not only degraded but also occasionally rearranged to thicken neighboring collagen fibrils. Importantly, we found a similarity of relationship between the enzyme-substrate interface structure and enzyme migration in collagen-collagenase and DNA-nuclease systems, which share a helical substrate structure, suggesting a common strategy in enzyme evolution. PMID:27373458

  15. Mapping octahedral tilts and polarization across a domain wall in BiFeO3 from Z-contrast STEM image atomic column shape analysis

    SciTech Connect

    Borisevich, Albina Y; Ovchinnikov, Oleg S; Chang, Hye Jung; Oxley, Mark P; Yu, P; Seidel, J; Eliseev, E. A.; Morozovska, A. N.; Ramesh, R.; Pennycook, Stephen J; Kalinin, Sergei V

    2010-01-01

    Oxygen octahedral tilts underpin the functionality of a large number of perovskite-based materials and heterostructures with competing order parameters. We show how a precise analysis of atomic column shapes in Z-contrast scanning transmission electron microscopy images can reveal polarization and octahedral tilt behavior across uncharged and charged domain walls in BiFeO3. This method is capable of visualizing octahedral tilts to much higher thicknesses than phase contrast imaging. We find that the octahedral tilt transition across a charged domain wall is atomically abrupt, while the associated polarization profile is diffuse (1.5-2 nm). Ginzburg-Landau theory then allows the relative contributions of polarization and the structural order parameters to the wall energy to be determined.

  16. Spin-polarized /sup 3/He nuclear targets and metastable /sup 4/He atoms by optical pumping with a tunable, Nd:YAP laser

    SciTech Connect

    Bohler, C.L.; Schearer, L.D.; Leduc, M.; Nacher, P.J.; Zachorowski, L.; Milner, R.G.; McKeown, R.D.; Woodward, C.E.

    1988-04-15

    Several Nd:YAP lasers were constructed which could be broadly tuned in the 1083-nm region which includes the helium 2/sup 3/S-2/sup 3/P transition, using a Lyot filter and thin, uncoated etalons within the laser cavity. 1 W of power could be extracted at 1083 nm through a 1% transmitting output coupler. This laser beam was used to optically pump metastable /sup 4/He and /sup 3/He 2/sup 3/S helium atoms in a weak discharge cell, spin polarizing the metastable ensemble. In a /sup 3/He cell the polarization is transferred to the nuclear spin system. A /sup 3/He target cell at 0.3 Torr was polarized to 52% in a few minutes. We describe the application of this system to the design of polarized targets for experiments in nuclear physics.

  17. Spin polarization and exchange coupling of Cu and Mn atoms in paramagnetic CuMn diluted alloys induced by a Co layer

    SciTech Connect

    Abes, M.; Arena, D.; Atkinson, D.; Tanner, B.K.; Charlton, T.R.; Langridge, S.; Hase, T.P.A.; Ali, M.; Marrows, C.H.; Hickey, B.J.; Neudert, Al; Hicken, R.J.; Wilkins, S.B.; Mirone, A.; Lebegue, S.

    2010-11-09

    Using the surface, interface, and element specificity of x-ray resonant magnetic scattering in combination with x-ray magnetic circular dichroism, we have spatially resolved the magnetic spin polarization, and the associated interface proximity effect, in a Mn-based high-susceptibility material close to a ferromagnetic Co layer. We have measured the magnetic polarization of Mn and Cu3d electrons in paramagnetic CuMn alloy layers in [Co/Cu(x)/CuMn/Cu(x)]{sub 20} multilayer samples with varying copper layer thicknesses from x=0 to 25 {angstrom}. The size of the Mn and CuL{sub 2,3} edge dichroism shows a decrease in the Mn-induced polarization for increasing copper thickness indicating the dominant interfacial nature of the Cu and Mn spin polarization. The Mn polarization is much higher than that of Cu. Evidently, the Mn moment is a useful probe of the local spin density. Mn atoms appear to be coupled antiferromagnetically with the Co layer below x = 10 {angstrom} and ferromagnetically coupled above. In contrast, the interfacial Cu atoms remain ferromagnetically aligned to the Co layer for all thicknesses studied.

  18. High-energy electron-energy spectra of atoms undergoing tunneling and barrier-suppression ionization by superintense linearly polarized laser radiation

    SciTech Connect

    Krainov, V.P.; Sofronov, A.V.

    2004-01-01

    The high-energy electron-energy spectra of atoms and atomic ions undergoing direct tunneling or barrier-suppression ionization by superintense linearly polarized femtosecond laser pulse are derived. The Landau-Dykhne adiabatic approximation is used. The new result is the simple analytic expression for the electron momentum spectrum along the polarization axis and along the other directions in the case of the relativistic quiver electron energies. The contribution from the direct tunneling ionization exceeds the contribution from the ionization occurring in the rescattering processes. The energy spectrum is independent of the laser frequency and of the nonrelativistic ionization potential of the atom (atomic ion) considered. The conclusions have been made that (1) the drift electron energy along the polarization axis is much greater than in other directions. (2) the energy distribution depends on the sign of the electron drift momentum along the propagation of laser radiation, and (3) the electron drift energy is the nonrelativistic quantity even when the quiver electron energy has high ultrarelativistic values.

  19. FAST TRACK COMMUNICATION: Generalized geometrical model for photoionization of polarized atoms: II. Magnetic dichroism in the 3p photoemission from the K 3p64s 2S1/2 ground state

    NASA Astrophysics Data System (ADS)

    Grum-Grzhimailo, A. N.; Cubaynes, D.; Heinecke, E.; Hoffmann, P.; Zimmermann, P.; Meyer, M.

    2010-10-01

    The generalized geometrical model for photoionization from polarized atoms is extended to include mixing of configurations in the initial atomic and/or the final photoion states. The theoretical results for angle-resolved linear and circular magnetic dichroism are in good agreement with new high-resolution photoelectron data for 3p-1 photoionization of potassium atoms polarized in the K 3p64s 2S1/2 ground state by laser optical pumping.

  20. Atomically smooth and homogeneously N-polar AlN film grown on silicon by alumination of Si{sub 3}N{sub 4}

    SciTech Connect

    Hu, Jiannan; Hao, Zhibiao; Niu, Lang; Yanxiong E,; Wang, Lai; Luo, Yi

    2013-04-08

    By using an alumination process of Si{sub 3}N{sub 4} at high temperature with aluminum flux irradiation for sufficient time, homogeneously N-polar and atomically smooth AlN film has been realized on silicon substrate with inversion domain suppressed to less than 3.0 Multiplication-Sign 10{sup 6} cm{sup -2} and root mean square surface roughness of {approx}0.4 nm. A general interface model is proposed to explain the mechanism of polarity determination. The sharp AlN(0001)/Si(111) interface exhibits 5:4 coincidence domain matching, resulting in an almost fully relaxed AlN film.

  1. VISIONS remote observations of a spatially-structured filamentary source of energetic neutral atoms near the polar cap boundary during an auroral substorm

    NASA Astrophysics Data System (ADS)

    Collier, Michael R.; Chornay, D.; Clemmons, J.; Keller, J. W.; Klenzing, J.; Kujawski, J.; McLain, J.; Pfaff, R.; Rowland, D.; Zettergren, M.

    2015-11-01

    We report initial results from the VISualizing Ion Outflow via Neutral atom imaging during a Substorm (VISIONS) rocket that flew through and near several regions of enhanced auroral activity and also sensed regions of ion outflow both remotely and directly. The observed neutral atom fluxes were largest at the lower energies and generally higher in the auroral zone than in the polar cap. In this paper, we focus on data from the latter half of the VISIONS trajectory when the rocket traversed the polar cap region. During this period, many of the energetic neutral atom spectra show a peak at 100 eV. Spectra with peaks around 100 eV are also observed in the Electrostatic Ion Analyzer (EIA) data consistent with these ions comprising the source population for the energetic neutral atoms. The EIA observations of this low energy population extend only over a few tens of km. Furthermore, the directionality of the arriving energetic neutral atoms is consistent with either this spatially localized source of energetic ions extending from as low as about 300 km up to above 600 km or a larger source of energetic ions to the southwest.

  2. VISIONS: Remote Observations of a Spatially-Structured Filamentary Source of Energetic Neutral Atoms near the Polar Cap Boundary During an Auroral Substorm

    NASA Technical Reports Server (NTRS)

    Collier, Michael R.; Chornay, D.; Clemmons, J.; Keller, J. W.; Klenzing, J.; Kujawski, J.; McLain, J.; Pfaff, R.; Rowland, D.; Zettergren, M.

    2015-01-01

    We report initial results from the VISualizing Ion Outflow via Neutral atom imaging during a Substorm (VISIONS) rocket that flew through and near several regions of enhanced auroral activity and also sensed regions of ion outflow both remotely and directly. The observed neutral atom fluxes were largest at the lower energies and generally higher in the auroral zone than in the polar cap. In this paper, we focus on data from the latter half of the VISIONS trajectory when the rocket traversed the polar cap region. During this period, many of the energetic neutral atom spectra show a peak at 100 electronvolts. Spectra with peaks around 100 electronvolts are also observed in the Electrostatic Ion Analyzer (EIA) data consistent with these ions comprising the source population for the energetic neutral atoms. The EIA observations of this low energy population extend only over a few tens of kilometers. Furthermore, the directionality of the arriving energetic neutral atoms is consistent with either this spatially localized source of energetic ions extending from as low as about 300 kilometers up to above 600 kilometers or a larger source of energetic ions to the southwest.

  3. Production, formation, and transport of high-brightness atomic hydrogen beam studies for the relativistic heavy ion collider polarized source upgrade

    NASA Astrophysics Data System (ADS)

    Kolmogorov, A.; Atoian, G.; Davydenko, V.; Ivanov, A.; Ritter, J.; Stupishin, N.; Zelenski, A.

    2014-02-01

    The RHIC polarized H- ion source had been successfully upgraded to higher intensity and polarization by using a very high brightness fast atomic beam source developed at BINP, Novosibirsk. In this source the proton beam is extracted by a four-grid multi-aperture ion optical system and neutralized in the H2 gas cell downstream from the grids. The proton beam is extracted from plasma emitter with a low transverse ion temperature of ˜0.2 eV which is formed by plasma jet expansion from the arc plasma generator. The multi-hole grids are spherically shaped to produce "geometrical" beam focusing. Proton beam formation and transport of atomic beam were experimentally studied at test bench.

  4. Production, formation, and transport of high-brightness atomic hydrogen beam studies for the relativistic heavy ion collider polarized source upgrade

    SciTech Connect

    Kolmogorov, A. Stupishin, N.; Atoian, G.; Ritter, J.; Zelenski, A.; Davydenko, V.; Ivanov, A.

    2014-02-15

    The RHIC polarized H{sup −} ion source had been successfully upgraded to higher intensity and polarization by using a very high brightness fast atomic beam source developed at BINP, Novosibirsk. In this source the proton beam is extracted by a four-grid multi-aperture ion optical system and neutralized in the H{sub 2} gas cell downstream from the grids. The proton beam is extracted from plasma emitter with a low transverse ion temperature of ∼0.2 eV which is formed by plasma jet expansion from the arc plasma generator. The multi-hole grids are spherically shaped to produce “geometrical” beam focusing. Proton beam formation and transport of atomic beam were experimentally studied at test bench.

  5. Production, formation, and transport of high-brightness atomic hydrogen beam studies for the relativistic heavy ion collider polarized source upgrade.

    PubMed

    Kolmogorov, A; Atoian, G; Davydenko, V; Ivanov, A; Ritter, J; Stupishin, N; Zelenski, A

    2014-02-01

    The RHIC polarized H(-) ion source had been successfully upgraded to higher intensity and polarization by using a very high brightness fast atomic beam source developed at BINP, Novosibirsk. In this source the proton beam is extracted by a four-grid multi-aperture ion optical system and neutralized in the H2 gas cell downstream from the grids. The proton beam is extracted from plasma emitter with a low transverse ion temperature of ∼0.2 eV which is formed by plasma jet expansion from the arc plasma generator. The multi-hole grids are spherically shaped to produce "geometrical" beam focusing. Proton beam formation and transport of atomic beam were experimentally studied at test bench. PMID:24593468

  6. Master equation theory applied to the redistribution of polarized radiation in the weak radiation field limit. III. Theory for the multilevel atom

    NASA Astrophysics Data System (ADS)

    Bommier, Véronique

    2016-06-01

    Context. We discuss the case of lines formed by scattering, which comprises both coherent and incoherent scattering. Both processes contribute to form the line profiles in the so-called second solar spectrum, which is the spectrum of the linear polarization of such lines observed close to the solar limb. However, most of the lines cannot be simply modeled with a two-level or two-term atom model, and we present a generalized formalism for this purpose. Aims: The aim is to obtain a formalism that is able to describe scattering in line centers (resonant scattering or incoherent scattering) and in far wings (Rayleigh/Raman scattering or coherent scattering) for a multilevel and multiline atom. Methods: The method is designed to overcome the Markov approximation, which is often performed in the atom-photon interaction description. The method was already presented in the two first papers of this series, but the final equations of those papers were for a two-level atom. Results: We present here the final equations generalized for the multilevel and multiline atom. We describe the main steps of the theoretical development, and, in particular, how we performed the series development to overcome the Markov approximation. Conclusions: The statistical equilibrium equations for the atomic density matrix and the radiative transfer equation coefficients are obtained with line profiles. The Doppler redistribution is also taken into account because we show that the statistical equilibrium equations must be solved for each atomic velocity class.

  7. Signatures of a conical intersection in photofragment distributions and absorption spectra: Photodissociation in the Hartley band of ozone

    SciTech Connect

    Picconi, David; Grebenshchikov, Sergy Yu.

    2014-08-21

    Photodissociation of ozone in the near UV is studied quantum mechanically in two excited electronic states coupled at a conical intersection located outside the Franck-Condon zone. The calculations, performed using recent ab initio PESs, provide an accurate description of the photodissociation dynamics across the Hartley/Huggins absorption bands. The observed photofragment distributions are reproduced in the two electronic dissociation channels. The room temperature absorption spectrum, constructed as a Boltzmann average of many absorption spectra of rotationally excited parent ozone, agrees with experiment in terms of widths and intensities of diffuse structures. The exit channel conical intersection contributes to the coherent broadening of the absorption spectrum and directly affects the product vibrational and translational distributions. The photon energy dependences of these distributions are strikingly different for fragments created along the adiabatic and the diabatic paths through the intersection. They can be used to reverse engineer the most probable geometry of the non-adiabatic transition. The angular distributions, quantified in terms of the anisotropy parameter β, are substantially different in the two channels due to a strong anticorrelation between β and the rotational angular momentum of the fragment O{sub 2}.

  8. Intermediate photofragment distributions as probes of non-adiabatic dynamics at conical intersections: application to the Hartley band of ozone.

    PubMed

    Picconi, David; Grebenshchikov, Sergy Yu

    2015-11-21

    Quantum dynamics at a reactive two-state conical intersection lying outside the Franck-Condon zone is studied for a prototypical reaction of ultraviolet photodissociation of ozone in the Hartley band. The focus is on the vibrational distributions in the two electronic states at intermediate interfragment distances near the intersection. Such intermediate distributions of strongly interacting photofragments contain unique information on the location and shape of the conical intersection. Multidimensional Landau-Zener modeling provides a framework to reverse engineer the molecular geometry-dependent Massey parameter of the intersection from the intermediate distributions. The conceptual approach is demonstrated for the intermediate O-O bond stretch distributions which become strongly inverted on adiabatic passage through the intersection. It is further demonstrated that intermediate distributions can be reconstructed from the photoemission spectrum of the dissociating molecule. The illustration, given using quantum mechanical calculations of resonance Raman profiles for ozone, completes a practicable cycle of conversion of intermediate distributions into topographic features of the conical intersection. PMID:26455514

  9. Polarization of Lyman-Alpha Radiation from Atomic Hydrogen Excited by Electron Impact form Near Threshold to 1800 eV

    NASA Technical Reports Server (NTRS)

    James, G. K.; Slevin, J. A.; Dziczek, D.; McConkey, J. W.; Bray, Igor

    1998-01-01

    The polarization of Lyman-a radiation, produced by electron-impact excitation of atomic hydrogen, has been measured over the extended energy range from near threshold to 1800 eV. Measurements were obtained in a crossed-beam experiment using a silica-reflection linear polarization analyzer in tandem with a vacuum-ultraviolet monochromator to isolate the emitted line radiation. Comparison with various theoretical calculations shows that the present experimental results are in good agreement with theory over the entire range of electron-impact energies and, in particular, are in excellent agreement with theoretical convergent-close-coupling (CCC) calculations performed in the present work. Our polarization data are significantly different from the previous experimental measurements of Ott, Kauppila, and Fite.

  10. The effect of atomic structure on interface spin-polarization of half-metallic spin valves: Co{sub 2}MnSi/Ag epitaxial interfaces

    SciTech Connect

    Nedelkoski, Zlatko; Hasnip, Philip J.; Kuerbanjiang, Balati; Higgins, Edward; Lazarov, Vlado K.; Sanchez, Ana M.; Bell, Gavin R.; Oogane, Mikihiko; Hirohata, Atsufumi

    2015-11-23

    Using density functional theory calculations motivated by aberration-corrected electron microscopy, we show how the atomic structure of a fully epitaxial Co{sub 2}MnSi/Ag interfaces controls the local spin-polarization. The calculations show clear difference in spin-polarization at Fermi level between the two main types: bulk-like terminated Co/Ag and Mn-Si/Ag interfaces. Co/Ag interface spin-polarization switches sign from positive to negative, while in the case of Mn-Si/Ag, it is still positive but reduced. Cross-sectional atomic structure analysis of Co{sub 2}MnSi/Ag interface, part of a spin-valve device, shows that the interface is determined by an additional layer of either Co or Mn. The presence of an additional Mn layer induces weak inverse spin-polarisation (−7%), while additional Co layer makes the interface region strongly inversely spin-polarized (−73%). In addition, we show that Ag diffusion from the spacer into the Co{sub 2}MnSi electrode does not have a significant effect on the overall Co{sub 2}MnSi /Ag performance.

  11. Lyman-alpha fluorescence from hydrogen photofragments of CH4 and H2O

    NASA Technical Reports Server (NTRS)

    Wu, C. Y. R.; Judge, D. L.

    1981-01-01

    The process of H-Lyman-alpha fluorescence produced through photodissociation of CH4 and H2O provides an example for the usefulness of the detection of fluorescence of dissociation fragments as an aid in identifying some high lying Rydberg states. In the first experiment reported, an electron storage ring synchrotron radiation source was used. The fluorescence produced was detected with a solar blind photomultiplier and a Cs photocathode with a spectral sensitivity in the wavelength range from 1050 to 1950 A. In the second experiment considered, an intense atomic line source was employed.

  12. Efficient production of polar molecular Bose-Einstein condensates via an all-optical R-type atom-molecule adiabatic passage

    NASA Astrophysics Data System (ADS)

    Qian, Jing; Zhou, Lu; Zhang, Keye; Zhang, Weiping

    2010-03-01

    We propose a scheme of 'R-type' photoassociative adiabatic passage (PAP) to create polar molecular condensates from two different species of ultracold atoms. Due to the presence of a quasi-coherent population trapping state in the scheme, it is possible to associate atoms into molecules with a low-power photoassociation (PA) laser. One remarkable advantage of our scheme is that a tunable atom-molecule coupling strength can be achieved by using a time-dependent PA field, which exhibits larger flexibility than using a tunable magnetic field. In addition, our results show that the PA intensity required in the 'R-type' PAP could be greatly reduced compared to that in a conventional 'Λ-type' one.

  13. Effects of the interior static polarization in photoionization of ``regular'' (A@C60) and ``giant'' (A@C240) endohedral atoms: A comparative study

    NASA Astrophysics Data System (ADS)

    Akiyama, Takehiro; Dolmatov, Valeriy

    2010-10-01

    Recently, photoionization of an atom A confined inside the C60 fullerene (A@C60) has come under a novel theoretical scrutiny by accounting for static relaxation of the system in response to ionization of the atom A, termed the interior static polarization effect [1]. In the present work, we explore how the impact might get altered with increasing size of the fullerene cage. ``Regular'' C60 and ``giant'' C240 cages with the Ne atom sitting at the center of a cage, i.e., Ne@C60 and Ne@C240, are chosen for the study. Both carbon cages are regarded as conducting spheres. They are simulated by the corresponding potentials of given inner radii, depths, and thickness [2]. The impact's significance is found to be about the same in both systems. It strongly alters the photoionization of the encaged atom near threshold as well as changes phases of associated confinement resonances. However, the photoionization spectrum of the encaged atom differs much stronger from that of the free atom with increasing size of the cage. [1] V. K. Dolmatov and S. T. Manson, Phys. Rev. A (in print). [2] V. K. Dolmatov, Adv. Quant. Chem., 58, 13 (2009).

  14. Anomalous elastic scattering of linearly polarized X-ray radiation by multicharged atomic ions in the range of the ionization threshold of the 1 s-shell

    NASA Astrophysics Data System (ADS)

    Hopersky, A. N.; Novikov, S. A.; Chuvenkov, V. V.

    2002-04-01

    The absolute values and shape of differential cross-section of the process of the anomalous elastic scattering for non-zero angle are investigated within non-relativistic approximation for linearly polarized X-ray radiation scattered by multicharged atomic ions Ne 6+ in the range of the ionization threshold of 1 s-shell. The many-particle effects of radial rearrangement of electron shells in the field of an inner 1 s-vacancy and the effect of vacancy stabilization are taken into account. The results of the work are predictions.

  15. Circularly polarized high harmonics generated by a bicircular field from inert atomic gases in the p state: A tool for exploring chirality-sensitive processes

    NASA Astrophysics Data System (ADS)

    Milošević, D. B.

    2015-10-01

    S -matrix theory of high-order harmonic generation (HHG) is generalized to multielectron atoms. In the multielectron case the harmonic power is expressed via a coherent sum of the time-dependent dipoles, while for the one-electron models a corresponding incoherent sum appears. This difference is important for the inert atomic gases having a p ground state as used in a recent HHG experiment with a bicircular field [Nat. Photonics 9, 99 (2015), 10.1038/nphoton.2014.293]. We investigate HHG by such a bicircular field, which consists of two coplanar counter-rotating circularly polarized fields of frequency r ω and s ω . Selection rules for HHG by a bicircular field are analyzed from the aspects of dynamical symmetry of the system, conservation of the projection of the angular momentum on a fixed quantization axis, and the quantum number of the initial and final atomic ground states. A distinction is made between the selection rules for atoms with closed [J. Phys. B 48, 171001 (2015), 10.1088/0953-4075/48/17/171001] and nonclosed shells. An asymmetry in emission of the left- and right-circularly polarized harmonics is found and explained by using a semiclassical model and the electron probability currents which are related to a nonzero magnetic quantum number. This asymmetry can be important for the application of such harmonics to the exploration of chirality-sensitive processes and for generation of elliptic or even circular attosecond pulse trains. Such attosecond pulse trains are analyzed for longer wavelengths than in Opt. Lett. 40, 2381 (2015), 10.1364/OL.40.002381, and for various field-component intensities.

  16. Doppler spectroscopy of hydrogen atoms from the photodissociation of saturated hydrocarbons and methyl halides at 157 nm

    SciTech Connect

    Tonokura, K.; Matsumi, Y.; Kawasaki, M. ); Kasatani, K. )

    1991-10-01

    Hydrocarbons (C{sub {ital n}}H{sub 2{ital n}+2}, {ital n}=3, 4, and 6) and methyl halides (CH{sub 3}{ital X}, {ital X}=Cl, Br, I) are photodissociated at 157 nm. The hydrogen atom photofragments are detected by a resonance-enhanced multiphoton ionization technique. The Doppler profiles of the hydrogen atoms from hydrocarbons are well represented by a Gaussian profile, while those from methyl halides by a mixture of a Gaussian and a non-Gaussian profiles. These Doppler profiles are interpreted assuming that (a) hot ethyl photofragments from hydrocarbons result in the formation of hydrogen atoms and (b) methyl halides undergo both direct and indirect photolytic scissions of the C---H bonds at 157 nm.

  17. Collisional properties of cold spin-polarized nitrogen gas: Theory, experiment, and prospects as a sympathetic coolant for trapped atoms and molecules

    SciTech Connect

    Tscherbul, T. V.; Dalgarno, A.; Klos, J.; Zygelman, B.; Pavlovic, Z.; Hummon, M. T.; Lu, H.-I.; Tsikata, E.; Doyle, J. M.

    2010-10-15

    We report a combined experimental and theoretical study of collision-induced dipolar relaxation in a cold spin-polarized gas of atomic nitrogen (N). We use buffer gas cooling to create trapped samples of {sup 14}N and {sup 15}N atoms with densities (5{+-}2)x10{sup 12} cm{sup -3} and measure their magnetic relaxation rates at milli-Kelvin temperatures. These measurements, together with rigorous quantum scattering calculations based on accurate ab initio interaction potentials for the {sup 7}{Sigma}{sub u}{sup +} electronic state of N{sub 2} demonstrate that dipolar relaxation in N+N collisions occurs at a slow rate of {approx}10{sup -13} cm{sup 3}/s over a wide range of temperatures (1 mK to 1 K) and magnetic fields (10 mT to 2 T). The calculated dipolar relaxation rates are insensitive to small variations of the interaction potential and to the magnitude of the spin-exchange interaction, enabling the accurate calibration of the measured N atom density. We find consistency between the calculated and experimentally determined rates. Our results suggest that N atoms are promising candidates for future experiments on sympathetic cooling of molecules.

  18. Relativistic effects on the nuclear magnetic shieldings of rare-gas atoms and halogen in hydrogen halides within relativistic polarization propagator theory

    NASA Astrophysics Data System (ADS)

    Gomez, Sergio S.; Maldonado, Alejandro; Aucar, Gustavo A.

    2005-12-01

    In this work an analysis of the electronic origin of relativistic effects on the isotropic dia- and paramagnetic contributions to the nuclear magnetic shielding σ(X ) for noble gases and heavy atoms of hydrogen halides is presented. All results were obtained within the 4-component polarization propagator formalism at different level of approach [random-phase approximation (RPA) and pure zeroth-order approximation (PZOA)], by using a local version of the DIRAC code. From the fact that calculations of diamagnetic contributions to σ within RPA and PZOA approaches for HX(X =Br,I,At) and rare-gas atoms are quite close each to other and the finding that the diamagnetic part of the principal propagator at the PZOA level can be developed as a series [S(Δ)], it was found that there is a branch of negative-energy "virtual" excitations that contribute with more than 98% of the total diamagnetic value even for the heavier elements, namely, Xe, Rn, I, and At. It contains virtual negative-energy molecular-orbital states with energies between -2mc2 and -4mc2. This fact can explain the excellent performance of the linear response elimination of small component (LR-ESC) scheme for elements up to the fifth row in the Periodic Table. An analysis of the convergency of S(Δ ) and its physical implications is given. It is also shown that the total contribution to relativistic effects of the innermost orbital (1s1/2) is by far the largest. For the paramagnetic contributions results at the RPA and PZOA approximations are similar only for rare-gas atoms. On the other hand, if the mass-correction contributions to σp are expressed in terms of atomic orbitals, a different pattern is found for 1s1/2 orbital contributions compared with all other s-type orbitals when the whole set of rare-gas atoms is considered.

  19. Effects of nitrogen dopants on the atomic step kinetics and electronic structures of O-polar ZnO

    NASA Astrophysics Data System (ADS)

    Wang, Hao; Zhan, Huahan; Zhou, Yinghui; Wu, Yaping; Chen, Xiaohang; Wang, Huiqiong; Kang, Junyong

    2016-02-01

    Oxygen-polar ZnO films are grown in step flow mode by molecular beam epitaxy. Driven by the step flow anisotropy, the growth leads to the occurrence of specific hexagonal pits in the surface. The specific pits are formed by interlacing steps of the {101&cmb.macr;4&cmb.macr;} facets, thus quenching the macroscopic dipole moment along the c-axis and satisfying the stabilization principles. Nitrogen (N) doping trials are then performed on the basis of the stable surface. In doping, growth remains in step flow mode but the step flow anisotropy vanishes, resulting in an obvious change of the surface morphology. Besides, a distinct acceptor state appears by in situ scanning tunneling spectroscopy analysis. First-principles calculations reveal that N readily substitutes for step-edge Zn and acts as NO2 adsorbed at the step edge. Desorption of the NO2 facilitates the formation of NO-VZn shallow acceptor complexes, which contributes to the appearance of the acceptor state. According to the peculiarities of N dopants on the O-polar surface, vicinal O-polar substrates (e.g., {101&cmb.macr;4&cmb.macr;} substrate) are promising in ZnO : N due to the easily achieved step flow growth and high density of step edges for N incorporation.

  20. Atomic polarizabilities

    SciTech Connect

    Safronova, M. S.; Mitroy, J.; Clark, Charles W.; Kozlov, M. G.

    2015-01-22

    The atomic dipole polarizability governs the first-order response of an atom to an applied electric field. Atomic polarization phenomena impinge upon a number of areas and processes in physics and have been the subject of considerable interest and heightened importance in recent years. In this paper, we will summarize some of the recent applications of atomic polarizability studies. A summary of results for polarizabilities of noble gases, monovalent, and divalent atoms is given. The development of the CI+all-order method that combines configuration interaction and linearized coupled-cluster approaches is discussed.

  1. Removal of Chromophore-Proximal Polar Atoms Decreases Water Content and Increases Fluorescence in a Near Infrared Phytofluor

    PubMed Central

    Lehtivuori, Heli; Bhattacharya, Shyamosree; Angenent-Mari, Nicolaas M.; Satyshur, Kenneth A.; Forest, Katrina T.

    2015-01-01

    Genetically encoded fluorescent markers have revolutionized cell and molecular biology due to their biological compatibility, controllable spatiotemporal expression, and photostability. To achieve in vivo imaging in whole animals, longer excitation wavelength probes are needed due to the superior ability of near infrared light to penetrate tissues unimpeded by absorbance from biomolecules or autofluorescence of water. Derived from near infrared-absorbing bacteriophytochromes, phytofluors are engineered to fluoresce in this region of the electromagnetic spectrum, although high quantum yield remains an elusive goal. An invariant aspartate residue is of utmost importance for photoconversion in native phytochromes, presumably due to the proximity of its backbone carbonyl to the pyrrole ring nitrogens of the biliverdin (BV) chromophore as well as the size and charge of the side chain. We hypothesized that the polar interaction network formed by the charged side chain may contribute to the decay of the excited state via proton transfer. Thus, we chose to further probe the role of this amino acid by removing all possibility for polar interactions with its carboxylate side chain by incorporating leucine instead. The resultant fluorescent protein, WiPhy2, maintains BV binding, monomeric status, and long maximum excitation wavelength while minimizing undesirable protoporphyrin IXα binding in cells. A crystal structure and time-resolved fluorescence spectroscopy reveal that water near the BV chromophore is excluded and thus validate our hypothesis that removal of polar interactions leads to enhanced fluorescence by increasing the lifetime of the excited state. This new phytofluor maintains its fluorescent properties over a broad pH range and does not suffer from photobleaching. WiPhy2 achieves the best compromise to date between high fluorescence quantum yield and long illumination wavelength in this class of fluorescent proteins. PMID:26636092

  2. Spin-orbit-induced spin-polarized surface states in one-atomic-layer Pb films on Si(111)

    NASA Astrophysics Data System (ADS)

    Lee, Hyungjun; Choi, Hyoung Joon

    2013-03-01

    As a route to spintronics without magnetism, spin-orbit coupling (SOC) generates and manipulates the spin-polarized carriers, thereby providing key ingredients for spin field-effect transistors. Along this line, we investigated the spin-orbit induced effects in Pb monolayers on Si(111) substrates, modeled by √{ 3} ×√{ 3} phase with Pb coverage of 4/3 ML, based on first-principles calculations with the inclusion of SOC. We focus on the electronic structures of surface states with characteristic Rashba-type spin splitting and spin texture as well as the charge flow pattern by calculating the current density distribution for the spin-polarized surface states. We also discuss our results on the difference from the spin splitting in the Shockley surface states on Au(111) surface. This work was supported by the NRF of Korea (Grant No. 2011-0018306), and computational resources have been provided by KISTI Supercomputing Center (Project No. KSC-2012-C2-14).

  3. Atomic Description of the Interface between Silica and Alumina in Aluminosilicates through Dynamic Nuclear Polarization Surface-Enhanced NMR Spectroscopy and First-Principles Calculations

    PubMed Central

    2015-01-01

    Despite the widespread use of amorphous aluminosilicates (ASA) in various industrial catalysts, the nature of the interface between silica and alumina and the atomic structure of the catalytically active sites are still subject to debate. Here, by the use of dynamic nuclear polarization surface enhanced NMR spectroscopy (DNP SENS) and density functional theory (DFT) calculations, we show that on silica and alumina surfaces, molecular aluminum and silicon precursors are, respectively, preferentially grafted on sites that enable the formation of Al(IV) and Si(IV) interfacial sites. We also link the genesis of Brønsted acidity to the surface coverage of aluminum and silicon on silica and alumina, respectively. PMID:26244620

  4. Atomic Description of the Interface between Silica and Alumina in Aluminosilicates through Dynamic Nuclear Polarization Surface-Enhanced NMR Spectroscopy and First-Principles Calculations.

    PubMed

    Valla, Maxence; Rossini, Aaron J; Caillot, Maxime; Chizallet, Céline; Raybaud, Pascal; Digne, Mathieu; Chaumonnot, Alexandra; Lesage, Anne; Emsley, Lyndon; van Bokhoven, Jeroen A; Copéret, Christophe

    2015-08-26

    Despite the widespread use of amorphous aluminosilicates (ASA) in various industrial catalysts, the nature of the interface between silica and alumina and the atomic structure of the catalytically active sites are still subject to debate. Here, by the use of dynamic nuclear polarization surface enhanced NMR spectroscopy (DNP SENS) and density functional theory (DFT) calculations, we show that on silica and alumina surfaces, molecular aluminum and silicon precursors are, respectively, preferentially grafted on sites that enable the formation of Al(IV) and Si(IV) interfacial sites. We also link the genesis of Brønsted acidity to the surface coverage of aluminum and silicon on silica and alumina, respectively. PMID:26244620

  5. Energetics of nonpolar and polar compounds in cationic, anionic, and nonionic micelles studied by all-atom molecular dynamics simulation combined with a theory of solutions.

    PubMed

    Date, Atsushi; Ishizuka, Ryosuke; Matubayasi, Nobuyuki

    2016-05-21

    Energetic analysis was conducted for nonpolar and polar solutes bound in a cationic micelle of dodecyl trimethyl ammonium bromide (DTAB), an anionic micelle of sodium dodecyl sulfate (SDS), and a nonionic micelle of tetraethylene glycol monododecyl ether (Brij30). All-atom molecular dynamics simulation was performed, and the free energies of binding the solutes in the hydrophobic-core and headgroup regions of the micelles were computed using the energy-representation method. It was found in all the micelles examined that aromatic naphthalene is preferably located more outward than aliphatic propane and that the polar solutes are localized at the interface of the hydrophobic and hydrophilic regions. The roles of the surfactant and water were then elucidated by decomposing the free energy into the contributions from the respective species. Water was observed to play a decisive role in determining the binding location of the solute, while the surfactant was found to be more important for the overall stabilization of the solute within the micelle. The effects of attractive and repulsive interactions of the solute with the surfactant and water were further examined, and their competition was analyzed in connection with the preferable location of the solute in the micellar system. PMID:27117093

  6. Electron Confinement Due to Stacking Control of Atomic Layers in SiC Polytypes: Roles of Floating States and Spontaneous Polarization

    NASA Astrophysics Data System (ADS)

    Matsushita, Yu-ichiro; Furuya, Shinnosuke; Oshiyama, Atsushi

    2014-09-01

    We report on first-principles total-energy electronic-structure calculations that clarify the stability and electronic structures of heterocrystalline superlattices consisting of SiC polytypes. The calculated local density of states unequivocally reveals substantial effects of spontaneous polarization in hexagonal polytypes. The polarization in the hexagonal region renders the band lineup slanted in real space along the stacking direction in the superlattice; furthermore, the counterpolarization in the cubic region makes it slanted in the reverse direction. We find that electrons are confined near the interface in the cubic region and that holes are under a negligible band offset. We also find that the slanted band lineup causes a downward (upward) shift of the conduction (valence) band edge and the band gap becomes narrower than that in the bulk polytype, offsetting the band gap increase due to the quantum confinement. The calculated Kohn-Sham orbitals of the conduction band bottoms distribute not at atomic sites but over interstitial channels in the 3C region, thus showing the floating nature common to sp3-bonded materials. It is found that the penetration of the floating states into the hexagonal region further modifies the band gap.

  7. Characterization of single transition metal oxide nanorods by combining atomic force microscopy and polarized micro-Raman spectroscopy

    NASA Astrophysics Data System (ADS)

    Najjar, Samar; Talaga, David; Coffinier, Yannick; Szunerits, Sabine; Boukherroub, Rabah; Servant, Laurent; Couzi, Michel; Bonhommeau, Sébastien

    2011-09-01

    Accurate chemical and structural characterization of free-standing zinc oxide (ZnO) and hematite (α-Fe2O3) nanorods has been carried out using an AFM/Raman correlative technique under polarized light. ZnO nanorods are found to be wurtzite-type single crystalline objects homogeneous in composition and grown along their principal axis of symmetry. Hematite specimens are rhombohedral corundum-type single crystals grown along a direction orthogonal to their principal axis of symmetry and exhibiting structural disorder. Certain hematite nanorods turn out to be very sensitive to laser heating. These studies reveal the high potential of the coupled AFM/Raman technique to examine the properties of these promising nanomaterials.

  8. Polarized negative ions

    SciTech Connect

    Haeberli, W.

    1981-04-01

    This paper presents a survey of methods, commonly in use or under development, to produce beams of polarized negative ions for injection into accelerators. A short summary recalls how the hyperfine interaction is used to obtain nuclear polarization in beams of atoms. Atomic-beam sources for light ions are discussed. If the best presently known techniques are incorporated in all stages of the source, polarized H/sup -/ and D/sup -/ beams in excess of 10 ..mu..A can probably be achieved. Production of polarized ions from fast (keV) beams of polarized atoms is treated separately for atoms in the H(25) excited state (Lamb-Shift source) and atoms in the H(1S) ground state. The negative ion beam from Lamb-Shift sources has reached a plateau just above 1 ..mu..A, but this beam current is adequate for many applications and the somewhat lower beam current is compensated by other desirable characteristics. Sources using fast polarized ground state atoms are in a stage of intense development. The next sections summarize production of polarized heavy ions by the atomic beam method, which is well established, and by optical pumping, which has recently been demonstrated to yield very large nuclear polarization. A short discussion of proposed ion sources for polarized /sup 3/He/sup -/ ions is followed by some concluding remarks.

  9. Physics with Polarized Nuclei.

    ERIC Educational Resources Information Center

    Thompson, William J.; Clegg, Thomas B.

    1979-01-01

    Discusses recent advances in polarization techniques, specifically those dealing with polarization of atomic nuclei, and how polarized beams and targets are produced. These techniques have greatly increased the scope of possible studies, and provided the tools for testing fundamental symmetries and the spin dependence of nuclear forces. (GA)

  10. Atomic structure of a polar ceramic/metal interface: {l_brace}222{r_brace}MgO/Cu

    SciTech Connect

    Benedek, R.; Shashkov, D.A.; Seidman, D.N.; Muller, D.A.; Silcox, J.; Chisholm, M.F.; Yang, L.H.

    1998-02-01

    {l_brace}222{r_brace}MgO/Cu is one of the most extensively characterized ceramic/metal interfaces, in view of the atom probe field ion microscopy, Z-contrast Scanning Transmission Electron Microscopy (STEM), and spatially resolved Electron energy loss spectroscopy (EELS) measurements performed by the present authors, as well as the high resolution electron microscopy (HREM) of this system by others. Atomistic simulations with local density functional theory (LDFT) and Molecular Dynamics (MD) have been performed to gain additional insight into the structure of this interface. This presentation describes an interface interatomic potential for {l_brace}222{r_brace}MgO/Cu derived from LDFT total energy calculations, and its application to structural properties, including the terminating species, the absence of dislocation standoff, and the symmetry of the interfacial dislocation network.

  11. Exploring Conceptual Frameworks of Models of Atomic Structures and Periodic Variations, Chemical Bonding, and Molecular Shape and Polarity: A Comparison of Undergraduate General Chemistry Students with High and Low Levels of Content Knowledge

    ERIC Educational Resources Information Center

    Wang, Chia-Yu; Barrow, Lloyd H.

    2013-01-01

    The purpose of the study was to explore students' conceptual frameworks of models of atomic structure and periodic variations, chemical bonding, and molecular shape and polarity, and how these conceptual frameworks influence their quality of explanations and ability to shift among chemical representations. This study employed a purposeful sampling…

  12. Electrons per atom ratio determination and Hume-Rothery electron concentration rule for P-based polar compounds studied by FLAPW-fourier calculations.

    PubMed

    Mizutani, Uichiro; Sato, Hirokazu; Inukai, Manabu; Nishino, Yoichi; Zijlstra, Eeuwe Sieds

    2015-02-01

    The extent to which reliable electrons per atom ratio, e/a, are determined and the validity of the Hume-Rothery stabilization mechanism are ensured upon increasing ionicity are studied by applying first-principles full potential linearized augmented plane wave (FLAPW)-Fourier band calculations to as many as 59 binary compounds formed by adding elements from periods 2-6 to phosphorus in group 15 of the Periodic Table. Van Arkel-Ketelaar triangle maps were constructed both by using the Allen electronegativity data and by using an energy difference between the center-of-gravity energies of FLAPW-derived s and p partial densities of states (DOSs) for the equiatomic compounds studied. The determination of e/a and the test of the interference condition, both of which play a key role in the Hume-Rothery stabilization mechanism, were reliably made for all intermetallic compounds, as long as the ionicity is less than 50%. In the A-P (A = Li, Na, K, Rb, and Cs) compounds with ionicity exceeding 50%, however, e/a determination becomes unstable, as reflected in its P concentration dependence. New Hume-Rothery electron concentration rules were theoretically found in two families of polar compounds: skutterudite compounds TMP(3), TMAs(3), and TMSb(3) (TM = Co, Ni, Rh, and Ir; cI32) with e/a = 4.34 and TM(3)P (TM = Cr, Mn, Fe, and Ni; tI32) with e/a = 2.20. PMID:25531024

  13. Polar catastrophe and the structure of KTa1-xNbxO₃ surfaces: Results from elastic and inelastic helium atom scattering

    SciTech Connect

    Flaherty, F. A.; Trelenberg, T. W.; Li, J. A.; Fatema, R.; Skofronick, J. G.; Van Winkle, D. H.; Safron, S. A.; Boatner, L. A.

    2015-07-13

    The structure and dynamics of cleaved (001) surfaces of potassium tantalates doped with niobium, KTa1-xNbxO₃ (KTN), with x ranging from 0% to 30%, were measured by helium atom scattering (HAS). Through HAS time-of-flight (TOF) experiments, a dispersionless branch (Einstein phonon branch) with energy of 13-14 meV was observed across the surface Brillouin zone in all samples. When this observation is combined with the results from earlier experimental and theoretical studies on these materials, a consistent picture of the stable surface structure emerges: After cleaving the single-crystal sample, the surface should be composed of equal areas of KO and TaO₂/NbO₂ terraces. The data, however, suggest that K⁺ and O²⁻ ions migrate from the bulk to the surface, forming a charged KO lattice that is neutralized primarily by additional K⁺ ions bridging pairs of surface oxygens. This structural and dynamic modification at the (001) surface of KTN appears due to its formally charged KO(-1) and TaO₂/NbO₂(+1) layers and avoids a “polar catastrophe.” This behavior is contrasted with the (001) surface behavior of the fluoride perovskite KMnF₃ with its electrically neutral KF and MnF₂ layers.

  14. Polar catastrophe and the structure of KTa1-xNbxO₃ surfaces: Results from elastic and inelastic helium atom scattering

    DOE PAGESBeta

    Flaherty, F. A.; Trelenberg, T. W.; Li, J. A.; Fatema, R.; Skofronick, J. G.; Van Winkle, D. H.; Safron, S. A.; Boatner, L. A.

    2015-07-13

    The structure and dynamics of cleaved (001) surfaces of potassium tantalates doped with niobium, KTa1-xNbxO₃ (KTN), with x ranging from 0% to 30%, were measured by helium atom scattering (HAS). Through HAS time-of-flight (TOF) experiments, a dispersionless branch (Einstein phonon branch) with energy of 13-14 meV was observed across the surface Brillouin zone in all samples. When this observation is combined with the results from earlier experimental and theoretical studies on these materials, a consistent picture of the stable surface structure emerges: After cleaving the single-crystal sample, the surface should be composed of equal areas of KO and TaO₂/NbO₂ terraces.more » The data, however, suggest that K⁺ and O²⁻ ions migrate from the bulk to the surface, forming a charged KO lattice that is neutralized primarily by additional K⁺ ions bridging pairs of surface oxygens. This structural and dynamic modification at the (001) surface of KTN appears due to its formally charged KO(-1) and TaO₂/NbO₂(+1) layers and avoids a “polar catastrophe.” This behavior is contrasted with the (001) surface behavior of the fluoride perovskite KMnF₃ with its electrically neutral KF and MnF₂ layers.« less

  15. Polar catastrophe and the structure of KTa1 xNbxO3 surfaces: Results from elastic and inelastic helium atom scattering

    SciTech Connect

    Flaherty, F. A.; Trelenberg, T. W.; Li, Jiefang; Skofronick, J. G.; Van Winkle, David; Safron, Sanford A.; Boatner, Lynn A

    2015-01-01

    The structure and dynamics of cleaved (001) surfaces of potassium tantalates doped with niobium, KTa1 xNbxO3 (KTN), with x ranging from 0% to 30%, were measured by helium atom scattering (HAS). Through HAS timeofflight (TOF) experiments, a dispersionless branch (Einstein phonon branch) with energy of 13 14 meV was observed across the surface Brillouin zone in all samples.When this observation is combined with the results from earlier experimental and theoretical studies on these materials, a consistent picture of the stable surface structure emerges: After cleaving the singlecrystal sample, the surface should be composed of equal areas of KO and TaO2/NbO2 terraces. The data, however, suggest that K+ and O2 ions migrate from the bulk to the surface, forming a charged KO lattice that is neutralized primarily by additional K+ ions bridging pairs of surface oxygens. This structural and dynamic modification at the (001) surface of KTN appears due to its formally charged KO( 1) and TaO2/NbO2(+1) layers and avoids a polar catastrophe. This behavior is contrasted with the (001) surface behavior of the fluoride perovskite KMnF3 with its electrically neutral KF and MnF2 layers.

  16. PREFACE: International Symposium on (e,2e), Double Photoionization and Related Topics & 15th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions

    NASA Astrophysics Data System (ADS)

    Martin, Nicholas L. S.; deHarak, Bruno A.

    2010-01-01

    From 30 July to 1 August 2009, over a hundred scientists from 18 countries attended the International Symposium on (e,2e), Double Photoionization and Related Topics and the 15th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions which were held at the W T Young Library of the University of Kentucky, USA. Both conferences were satellite meetings of the XXVI International Conference on Photonic, Electronic and Atomic Collisions (ICPEAC) held in Kalamazoo, Michigan, USA, 21-28 July 2009. These symposia covered a broad range of experimental and theoretical topics involving excitation, ionization (single and multiple), and molecular fragmentation, of a wide range of targets by photons and charged particles (polarized and unpolarized). Atomic targets ranged from hydrogen to the heavy elements and ions, while molecular targets ranged from H2 to large molecules of biological interest. On the experimental front, cold target recoil ion momentum spectroscopy (COLTRIMS), also known as the Reaction Microscope because of the complete information it gives about a wide variety of reactions, is becoming commonplace and has greatly expanded the ability of researchers to perform previously inaccessible coincidence experiments. Meanwhile, more conventional spectrometers are also advancing and have been used for increasingly sophisticated and exacting measurements. On the theoretical front great progress has been made in the description of target states, and in the scattering calculations used to describe both simple and complex reactions. The international nature of collaborations between theorists and experimentalists is exemplified by, for example, the paper by Ren et al which has a total of 13 authors of whom the experimental group of six is from Heidelberg, Germany, one theoretical group is from Australia, with the remainder of the theoreticians coming from several different institutions in the United States. A total of 52 invited talks and

  17. Sources of polarized negative ions: progress and prospects

    SciTech Connect

    Haeberli, W.

    1980-01-01

    A summary of recent progress in the art of producing beams of polarized ions is given. In all sources of polarized ions, one first produces (or selects) neutral atoms which are polarized in electron spin. Those types of sources which use a beam of thermal polarized hydrogen atoms are discussed. Progress made in the preparation of the atomic beam and the methods used to convert the neutral atoms to polarized ions is summarized. The second type of source discussed is based on fast (keV) polarized hydrogen atoms. Conversion to negative ions is very simple because one only needs to pass the fast atoms through a suitable charge exchange medium (gas or vapor). However, the production of the polarized atoms is more difficult in this case. The proposal to employ polarized alkali vapor to form a beam of polarized fast H atoms, where the polarized alkali atoms are produced either by an atomic beam apparatus or by optical pumping is discussed. (WHK)

  18. Power and polarization dependences of ultra-narrow electromagnetically induced absorption (EIA) spectra of 85 Rb atoms in degenerate two-level system

    NASA Astrophysics Data System (ADS)

    Qureshi, Muhammad Mohsin; Rehman, Hafeez Ur; Noh, Heung-Ryoul; Kim, Jin-Tae

    2016-05-01

    We have investigated ultra-narrow EIA spectral features with respect to variations of polarizations and powers of pump laser beam in a degenerate two-level system of the transition of 85 Rb D2 transition line. Polarizations of the probe laser beam in two separate experiments were fixed at right circular and horizontal linear polarizations, respectively while the polarizations of the pump lasers were varied from initial polarizations same as the probe laser beams to orthogonal to probe polarizations. One homemade laser combined with AOMs was used to the pump and probe laser beams instead of two different lasers to overcome broad linewidths of the homemade lasers. Theoretically, probe absorption coefficients have been calculated from optical Bloch equations of the degenerate two level system prepared by a pump laser beam. In the case of the circular polarization, EIA signal was obtained as expected theoretically although both pump and probe beams have same polarization. The EIA signal become smaller as power increases and polarizations of the pump and probe beams were same. When the polarization of the pump beam was linear polarization, maximum EIA signal was obtained theoretically and experimentally. Experimental EIA spectral shapes with respect to variations of the pump beam polarization shows similar trends as the theoretical results.

  19. Polarization of metastable 129Xe

    NASA Astrophysics Data System (ADS)

    Xia, Tian; Morgan, Steven; Jau, Yuan-Yu; Happer, William

    2008-05-01

    We have measured atomic polarization of metastable 129Xe in a pyrex cell by optical pumping, while metastability exchange optical pumping of 3He is routinely done. The atomic polarization of metastable Xe is on the order of 10%. Metastable xenon is created by electrodeless rf discharge. The hyperfine transition of metastable 129Xe is observed by microwave excitation. Atomic polarization can be demonstrated by comparison of the intensities of the transitions between different Zeeman sublevels, while pumping a specific optical transition of metastable Xe with circularly polarized light. This work offers insight into attempts to polarize 129Xe nuclei by metastability exchange optical pumping.

  20. Analyzing velocity map images to distinguish the primary methyl photofragments from those produced upon C-Cl bond photofission in chloroacetone at 193 nm.

    PubMed

    Alligood, Bridget W; Straus, Daniel B; Butler, Laurie J

    2011-07-21

    We use a combination of crossed laser-molecular beam scattering experiments and velocity map imaging experiments to investigate the three primary photodissociation channels of chloroacetone at 193 nm: C-Cl bond photofission yielding CH(3)C(O)CH(2) radicals, C-C bond photofission yielding CH(3)CO and CH(2)Cl products, and C-CH(3) bond photofission resulting in CH(3) and C(O)CH(2)Cl products. Improved analysis of data previously reported by our group quantitatively identifies the contribution of this latter photodissociation channel. We introduce a forward convolution procedure to identify the portion of the signal, derived from the methyl image, which results from a two-step process in which C-Cl bond photofission is followed by the dissociation of the vibrationally excited CH(3)C(O)CH(2) radicals to CH(3) + COCH(2). Subtracting this from the total methyl signal identifies the methyl photofragments that result from the CH(3) + C(O)CH(2)Cl photofission channel. We find that about 89% of the chloroacetone molecules undergo C-Cl bond photofission to yield CH(3)C(O)CH(2) and Cl products; approximately 8% result in C-C bond photofission to yield CH(3)CO and CH(2)Cl products, and the remaining 2.6% undergo C-CH(3) bond photofission to yield CH(3) and C(O)CH(2)Cl products. PMID:21786998

  1. Fluorescence Excitation Spectra of Photo-Fragmented Nitrobenzene Using a Picosecond Laser: Potential Evidence for no Produced by Two Distinct Channels.

    NASA Astrophysics Data System (ADS)

    Lue, Christopher J.; Tanjaroon, Chakree; Johnson, J. Bruce; Reeve, Scott W.; Allen, Susan D.

    2013-06-01

    Upon absorption of a UV photon, nitrobenzene can dissociate into C_6H_5O and NO through two different mechanisms. Evidence for these mechanisms was obtained from velocity map imaging (VMI) studies and theoretical calculations. VMI experiments showed NO produced with two distinct rotational distributions, which the calculations explained as a fast and a slow channel for NO production. We have recorded high resolution fluorescence excitation spectra of the NO resulting from photo-fragmented nitrobenzene using a pulsed picosecond tunable laser (pulse width ≈ 15 ps) by means of a two-color process. In the two-color process, photons of a particular energy dissociated the nitrobenzene while photons of a different energy probed the A^2Σ^+← X^2Π_{(1/2,3/2)} NO band system between 225-260 nm. This laser system allowed us to vary the delay between the photolysis and excitation pulses. At longer delays (>1 ns), we observed an increase in the population of NO, which may be evidence that at least two photolysis channels produce NO. We present the spectra we recorded at various photolysis/probe delays ranging from 0.025 to 1.5 ns. The spectral subtraction method we used to observe the production increase is introduced. Hause, M. L.; Herath, N.; Zhu, R.; Lin, M. C. and Suits, A. G. Nat Chem, Nature Publishing Group, 2011, 3, 932-937

  2. Optical atomic magnetometer

    DOEpatents

    Budker, Dmitry; Higbie, James; Corsini, Eric P

    2013-11-19

    An optical atomic magnetometers is provided operating on the principles of nonlinear magneto-optical rotation. An atomic vapor is optically pumped using linearly polarized modulated light. The vapor is then probed using a non-modulated linearly polarized light beam. The resulting modulation in polarization angle of the probe light is detected and used in a feedback loop to induce self-oscillation at the resonant frequency.

  3. Atomic magnetometer

    DOEpatents

    Schwindt, Peter; Johnson, Cort N.

    2012-07-03

    An atomic magnetometer is disclosed which uses a pump light beam at a D1 or D2 transition of an alkali metal vapor to magnetically polarize the vapor in a heated cell, and a probe light beam at a different D2 or D1 transition to sense the magnetic field via a polarization rotation of the probe light beam. The pump and probe light beams are both directed along substantially the same optical path through an optical waveplate and through the heated cell to an optical filter which blocks the pump light beam while transmitting the probe light beam to one or more photodetectors which generate electrical signals to sense the magnetic field. The optical waveplate functions as a quarter waveplate to circularly polarize the pump light beam, and as a half waveplate to maintain the probe light beam linearly polarized.

  4. Review of Polarized Ion Sources

    NASA Astrophysics Data System (ADS)

    Zelenski, A.

    2016-02-01

    Recent progress in polarized ion sources development is reviewed. New techniques for production of polarized H‑ ion (proton), D‑ (D+) and 3He++ ion beams will be discussed. A novel polarization technique was successfully implemented for the upgrade of the RHIC polarized H‑ ion source to higher intensity and polarization. In this technique, a proton beam inside the high magnetic field solenoid is produced by ionization of the atomic hydrogen beam (from an external source) in the He-gas ionizer cell. Polarized electron capture from the optically-pumped Rb vapor further produces proton polarization (Optically Pumped Polarized Ion Source technique). The upgraded source reliably delivered beam for the 2013 polarized run in RHIC at S = 510 GeV. This was a major factor contributing to RHIC polarization increase to over 60 % for colliding beams. Feasibility studies of a new polarization technique for polarized 3He++ source based on BNL Electron Beam Ion Source is also discussed.

  5. Polarization transfer of bremsstrahlung arising from spin-polarized electrons.

    PubMed

    Märtin, R; Weber, G; Barday, R; Fritzsche, Y; Spillmann, U; Chen, W; DuBois, R D; Enders, J; Hegewald, M; Hess, S; Surzhykov, A; Thorn, D B; Trotsenko, S; Wagner, M; Winters, D F A; Yerokhin, V A; Stöhlker, Th

    2012-06-29

    We report on a study of the polarization transfer between transversely polarized incident electrons and the emitted x rays for electron-atom bremsstrahlung. By means of Compton polarimetry we performed for the first time an energy-differential measurement of the complete properties of bremsstrahlung emission related to linear polarization, i.e., the degree of linear polarization as well as the orientation of the polarization axis. For the high-energy end of the bremsstrahlung continuum the experimental results for both observables show a high sensitivity on the initial electron spin polarization and prove that the polarization orientation is virtually independent of the photon energy. PMID:23004992

  6. Analyzing velocity map images to distinguish the primary methyl photofragments from those produced upon C-Cl bond photofission in chloroacetone at 193 nm

    SciTech Connect

    Alligood, Bridget W.; Straus, Daniel B.; Butler, Laurie J.

    2011-07-21

    We use a combination of crossed laser-molecular beam scattering experiments and velocity map imaging experiments to investigate the three primary photodissociation channels of chloroacetone at 193 nm: C-Cl bond photofission yielding CH{sub 3}C(O)CH{sub 2} radicals, C-C bond photofission yielding CH{sub 3}CO and CH{sub 2}Cl products, and C-CH{sub 3} bond photofission resulting in CH{sub 3} and C(O)CH{sub 2}Cl products. Improved analysis of data previously reported by our group quantitatively identifies the contribution of this latter photodissociation channel. We introduce a forward convolution procedure to identify the portion of the signal, derived from the methyl image, which results from a two-step process in which C-Cl bond photofission is followed by the dissociation of the vibrationally excited CH{sub 3}C(O)CH{sub 2} radicals to CH{sub 3}+ COCH{sub 2}. Subtracting this from the total methyl signal identifies the methyl photofragments that result from the CH{sub 3}+ C(O)CH{sub 2}Cl photofission channel. We find that about 89% of the chloroacetone molecules undergo C-Cl bond photofission to yield CH{sub 3}C(O)CH{sub 2} and Cl products; approximately 8% result in C-C bond photofission to yield CH{sub 3}CO and CH{sub 2}Cl products, and the remaining 2.6% undergo C-CH{sub 3} bond photofission to yield CH{sub 3} and C(O)CH{sub 2}Cl products.

  7. The Physics of Polarization

    NASA Astrophysics Data System (ADS)

    Degl'Innocenti, Egidio Landi

    2015-10-01

    The introductory lecture that has been delivered at this Symposium is a condensed version of an extended course held by the author at the XII Canary Island Winter School from November 13 to November 21, 2000. The full series of lectures can be found in Landi Degl'Innocenti (2002). The original reference is organized in 20 Sections that are here itemized: 1. Introduction, 2. Description of polarized radiation, 3. Polarization and optical devices: Jones calculus and Muller matrices, 4. The Fresnel equations, 5. Dichroism and anomalous dispersion, 6. Polarization in everyday life, 7. Polarization due to radiating charges, 8. The linear antenna, 9. Thomson scattering, 10. Rayleigh scattering, 11. A digression on Mie scattering, 12. Bremsstrahlung radiation, 13. Cyclotron radiation, 14. Synchrotron radiation, 15. Polarization in spectral lines, 16. Density matrix and atomic polarization, 17. Radiative transfer and statistical equilibrium equations, 18. The amplification condition in polarized radiative transfer, and 19. Coupling radiative transfer and statistical equilibrium equations.

  8. Towards Polarized Antiprotons at FAIR

    SciTech Connect

    Rathmann, Frank

    2007-06-13

    Understanding the interplay of the nuclear interaction with polarized protons and the electromagnetic interaction with polarized electrons in polarized atoms is crucial to progress towards the PAX goal to eventually produce stored polarized antiproton beams at FAIR. Presently, there exist two competing theoretical scenarios: one with substantial spin filtering of (anti)protons by atomic electrons, and a second one suggesting a self-cancellation of the electron contribution to spin filtering. After a brief review of the PAX physics case for polarized antiprotons at FAIR, a detailed discussion of future investigations, including spin-filtering experiments at COSY-Juelich and at the AD of CERN is presented.

  9. Measurements of Excitation Functions and Line Polarizations for Electron Impact Excitation of the n = 2, 3 States of Atomic Hydrogen in the Energy Range 11 - 2000 eV

    NASA Technical Reports Server (NTRS)

    James, G. K.; Ajello, J. M.; Kanik, I.; Slevin, J.; Franklin, B.; Shemansky, D.

    1993-01-01

    The electron-atomic hydrogen scattering system is an important testing ground for theoretical models and has received a great deal of attention from experimentalists and theoreticians alike over the years. A complete description of the excitation process requires a knowledge of many different parameters, and experimental measurements of these parameters have been performed in various laboratories around the world. As far as total cross section data are concerned it has been noted that the discrepancy between the data of Long et al. and Williams for n = 2 excitations needs to be resolved in the interests of any further refinement of theory. We report new measurements of total cross sections and atomic line polarizations for both n=2 and n=3 excitations at energies from threshold to 2000 eV...

  10. Polarization and electronic excitation in nonreactive collisions: Basic formulation for quantum calculations of collisions between /sup 2/P-state alkali-metal atoms and H/sub 2/ or D/sub 2/

    SciTech Connect

    Baylis, W.E.; Pascale, J.; Rossi, F.

    1987-11-01

    The inelastic scattering of two structured systems: for example, an excited atom and a molecule: is considered in the case of nonreactive collisions. Explicit formulas are presented for cross sections corresponding to transitions between arbitrary eigenstates of the two isolated systems. These formulas are then used to derive cross sections for polarization transfer and multipole relaxation in one system when the other system is unpolarized. Both space-fixed and body-fixed formulations are given. Explicit matrix elements are worked out for interactions such as occur between model alkali-metal atoms and rigid-rotor diatomic molecules. An effective interaction method is also discussed and related to an adiabatic-state approach.

  11. Giant light enhancement in atomic clusters

    SciTech Connect

    Gadomsky, O. N. Gadomskaya, I. V.; Altunin, K. K.

    2009-07-15

    We show that the polarizing effect of the atoms in an atomic cluster can lead to full compensation of the radiative damping of excited atomic states, a change in the sign of the dispersion of the atomic polarizability, and giant light enhancement by the atomic cluster.

  12. Kinetic evidence for the formation of discrete 1,4-dehydrobenzene intermediates. Trapping by inter- and intramolecular hydrogen atom transfer and observation of high-temperature CIDNP (chemically induced dynamic nuclear polarization). [Chemically induced dynamic nuclear polarization

    SciTech Connect

    Lockhart, T.P.; Comita, P.B.; Bergman, R.G.

    1981-07-15

    Upon being heated, alkyl-substituted cis-1,2-diethynyl olefins undergo cyclization to yield reactive 1,4-dehydrobenzenes; the products isolated may be derived from either unimolecular or bimolecular reactions of the intermediate. (Z)-4,5-Diethynyl-4-octene (4) undergoes rearrangement to yield 2,3-di-n-propyl-1,4-dehydrobenzene (17). Solution pyrolysis of 4 in inert aromatic solvents produces three unimolecular products, (Z)-dodeca-4,8-diyn-6-ene (7), benzocycloctene (9), and o-allyl-n-propylbenzene (10), in high yield. When 1,4-cyclohexadiene is added to the pyrolysis solution as a trapping agent high yields of the reduced product o-di-n-propylbenzene (12) are obtained. The kinetics of solution pyrolysis of 4 in the presence and absence of trapping agent pyl-1,4-dehydrobenzene is a discrete intermediate on the pathway leading to products. When the reaction was run in the heated probe of an NMR spectrometer, chemically induced dynamic nuclear polarization was observed in 10. This observation, along with kinetic and chemical trapping evidence, indicates the presence of two additional intermediates, formed from 17 by sequential intramolecular (1,5) hydrogen transfer, on the pathway to products. The observation of CIDNP, coupled with the reactivity exhibited by 17 and the other two intermediates, implicates a biradical description of these molecules.

  13. Accurate adiabatic singlet-triplet gaps in atoms and molecules employing the third-order spin-flip algebraic diagrammatic construction scheme for the polarization propagator.

    PubMed

    Lefrancois, Daniel; Rehn, Dirk R; Dreuw, Andreas

    2016-08-28

    For the calculation of adiabatic singlet-triplet gaps (STG) in diradicaloid systems the spin-flip (SF) variant of the algebraic diagrammatic construction (ADC) scheme for the polarization propagator in third order perturbation theory (SF-ADC(3)) has been applied. Due to the methodology of the SF approach the singlet and triplet states are treated on an equal footing since they are part of the same determinant subspace. This leads to a systematically more accurate description of, e.g., diradicaloid systems than with the corresponding non-SF single-reference methods. Furthermore, using analytical excited state gradients at ADC(3) level, geometry optimizations of the singlet and triplet states were performed leading to a fully consistent description of the systems, leading to only small errors in the calculated STGs ranging between 0.6 and 2.4 kcal/mol with respect to experimental references. PMID:27586899

  14. Attaching an alkali metal atom to an alkaline earth metal oxide (BeO, MgO, or CaO) yields a triatomic metal oxide with reduced ionization potential and redirected polarity.

    PubMed

    Nowiak, Grzegorz; Skurski, Piotr; Anusiewicz, Iwona

    2016-04-01

    The existence of a series of neutral triatomic metal oxides MON and their corresponding cations MON (+) (M = Be, Mg, Ca; N = Li, Na, K) was postulated and verified theoretically using ab initio methods at the CCSD(T)/6-311+G(3df)//MP2/6-311+G(3df) level of theory. The calculations revealed that the vertical ionization potentials (IPs) of the MON radicals (calculated using the outer-valence Green's function technique (OVGF) with the 6-311+G(3df) basis set) were ca. 2-3 eV smaller than the IPs of the corresponding MO and NO systems or that of the isolated M atom. Population analysis of the neutral triatomic MON molecules and their corresponding MO counterparts indicated that the attachment of an alkali metal atom to any oxide MO (BeO, MgO, CaO) reverses its polarity, which manifests itself as the redirection of the dipole moment vector. PMID:26994021

  15. Components of the Bond Energy in Polar Diatomic Molecules, Radicals, and Ions Formed by Group-1 and Group-2 Metal Atoms.

    PubMed

    Yu, Haoyu; Truhlar, Donald G

    2015-07-14

    element, electron affinity of the electronegative bonding partner (EA), atomic excitation energy (EE) to prepare the valence states of the interacting partners, and interaction energy (IE) of the valence-prepared states. Adding Hartree-Fock exchange helps to obtain better results for atomic excitation energy, and this leads to improvements in getting the right answer for the right reason. The following functionals are singled out for reasonably good performance on all three of bond distance, BDE, and dipole moment: B97-1, B97-3, MPW1B95, M05, M06, M06-2X, M08-SO, N12-SX, O3LYP, TPSS, τ-HCTHhyb, and GAM; all but two (TPSS and GAM) of these functionals are hybrid functionals. PMID:26575734

  16. Measuring Gravitation Using Polarization Spectroscopy

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey; Yu, Nan; Maleki, Lute

    2004-01-01

    A proposed method of measuring gravitational acceleration would involve the application of polarization spectroscopy to an ultracold, vertically moving cloud of atoms (an atomic fountain). A related proposed method involving measurements of absorption of light pulses like those used in conventional atomic interferometry would yield an estimate of the number of atoms participating in the interferometric interaction. The basis of the first-mentioned proposed method is that the rotation of polarization of light is affected by the acceleration of atoms along the path of propagation of the light. The rotation of polarization is associated with a phase shift: When an atom moving in a laboratory reference interacts with an electromagnetic wave, the energy levels of the atom are Doppler-shifted, relative to where they would be if the atom were stationary. The Doppler shift gives rise to changes in the detuning of the light from the corresponding atomic transitions. This detuning, in turn, causes the electromagnetic wave to undergo a phase shift that can be measured by conventional means. One would infer the gravitational acceleration and/or the gradient of the gravitational acceleration from the phase measurements.

  17. The RHIC polarized H- ion source

    NASA Astrophysics Data System (ADS)

    Zelenski, A.; Atoian, G.; Raparia, D.; Ritter, J.; Steski, D.

    2016-02-01

    A novel polarization technique had been successfully implemented for the Relativistic Heavy Ion Collider (RHIC) polarized H- ion source upgrade to higher intensity and polarization. In this technique, a proton beam inside the high magnetic field solenoid is produced by ionization of the atomic hydrogen beam (from external source) in the He-gaseous ionizer cell. Further proton polarization is produced in the process of polarized electron capture from the optically pumped Rb vapor. The use of high-brightness primary beam and large cross sections of charge-exchange cross sections resulted in production of high intensity H- ion beam of 85% polarization. The source very reliably delivered polarized beam in the RHIC Run-2013 and Run-2015. High beam current, brightness, and polarization resulted in 75% polarization at 23 GeV out of Alternating Gradient Synchrotron (AGS) and 60%-65% beam polarization at 100-250 GeV colliding beams in RHIC.

  18. The RHIC polarized H⁻ ion source.

    PubMed

    Zelenski, A; Atoian, G; Raparia, D; Ritter, J; Steski, D

    2016-02-01

    A novel polarization technique had been successfully implemented for the Relativistic Heavy Ion Collider (RHIC) polarized H(-) ion source upgrade to higher intensity and polarization. In this technique, a proton beam inside the high magnetic field solenoid is produced by ionization of the atomic hydrogen beam (from external source) in the He-gaseous ionizer cell. Further proton polarization is produced in the process of polarized electron capture from the optically pumped Rb vapor. The use of high-brightness primary beam and large cross sections of charge-exchange cross sections resulted in production of high intensity H(-) ion beam of 85% polarization. The source very reliably delivered polarized beam in the RHIC Run-2013 and Run-2015. High beam current, brightness, and polarization resulted in 75% polarization at 23 GeV out of Alternating Gradient Synchrotron (AGS) and 60%-65% beam polarization at 100-250 GeV colliding beams in RHIC. PMID:26932068

  19. Atomic orientation following predissociation of the C {sup 3}{Pi}{sub g} Rydberg state of molecular oxygen

    SciTech Connect

    Gilchrist, A. J.; Ritchie, G. A. D.

    2013-06-07

    (2 + 1) resonance enhanced multiphoton ionization in combination with time-of-flight mass spectroscopy (TOF-MS) has been used to detect both the O({sup 3}P) and O({sup 1}D) fragments produced as a result of predissociation of the C {sup 3}{Pi}{sub g} (v= 0) and (v= 1) Rydberg states of O{sub 2}, accessed via two-photon absorption from the ground X {sup 3}{Sigma}{sub g}{sup -} state. In particular, TOF profiles have been recorded at various fixed two-photon absorption wavelengths within the two bands, with circular polarized probe laser light used to probe the angular momentum orientation of these photofragments. All photofragments are found to display coherent orientation resulting from interference between two possible two-photon absorption pathways. The measured orientation is affected by rotational depolarization due to the long lifetime of the excited C state; once this effect is accounted for the orientation is found to be nearly constant over all dissociation wavelengths. The origin of the coherent orientation is attributed to two-photon absorption to different spin-orbit components of the C state.

  20. Polarization developments

    SciTech Connect

    Prescott, C.Y.

    1993-07-01

    Recent developments in laser-driven photoemission sources of polarized electrons have made prospects for highly polarized electron beams in a future linear collider very promising. This talk discusses the experiences with the SLC polarized electron source, the recent progress with research into gallium arsenide and strained gallium arsenide as a photocathode material, and the suitability of these cathode materials for a future linear collider based on the parameters of the several linear collider designs that exist.

  1. Neuronal polarization.

    PubMed

    Takano, Tetsuya; Xu, Chundi; Funahashi, Yasuhiro; Namba, Takashi; Kaibuchi, Kozo

    2015-06-15

    Neurons are highly polarized cells with structurally and functionally distinct processes called axons and dendrites. This polarization underlies the directional flow of information in the central nervous system, so the establishment and maintenance of neuronal polarization is crucial for correct development and function. Great progress in our understanding of how neurons establish their polarity has been made through the use of cultured hippocampal neurons, while recent technological advances have enabled in vivo analysis of axon specification and elongation. This short review and accompanying poster highlight recent advances in this fascinating field, with an emphasis on the signaling mechanisms underlying axon and dendrite specification in vitro and in vivo. PMID:26081570

  2. Polarization Aberrations

    NASA Technical Reports Server (NTRS)

    Mcguire, James P., Jr.; Chipman, Russell A.

    1990-01-01

    The analysis of the polarization characteristics displayed by optical systems can be divided into two categories: geometrical and physical. Geometrical analysis calculates the change in polarization of a wavefront between pupils in an optical instrument. Physical analysis propagates the polarized fields wherever the geometrical analysis is not valid, i.e., near the edges of stops, near images, in anisotropic media, etc. Polarization aberration theory provides a starting point for geometrical design and facilitates subsequent optimization. The polarization aberrations described arise from differences in the transmitted (or reflected) amplitudes and phases at interfaces. The polarization aberration matrix (PAM) is calculated for isotropic rotationally symmetric systems through fourth order and includes the interface phase, amplitude, linear diattenuation, and linear retardance aberrations. The exponential form of Jones matrices used are discussed. The PAM in Jones matrix is introduced. The exact calculation of polarization aberrations through polarization ray tracing is described. The report is divided into three sections: I. Rotationally Symmetric Optical Systems; II. Tilted and Decentered Optical Systems; and Polarization Analysis of LIDARs.

  3. Collisional decoherence of polar molecules

    NASA Astrophysics Data System (ADS)

    Walter, Kai; Stickler, Benjamin A.; Hornberger, Klaus

    2016-06-01

    The quantum state of motion of a large and rotating polar molecule can lose coherence through the collisions with gas atoms. We show how the associated quantum master equation for the center of mass can be expressed in terms of the orientationally averaged differential and total scattering cross sections, for which we provide approximate analytic expressions. The master equation is then utilized to quantify collisional decoherence in a interference experiment with polar molecules.

  4. Polar Bear

    USGS Publications Warehouse

    Amstrup, S.D.; DeMaster

    1988-01-01

    Polar bears are long-lived, late-maturing carnivores that have relatively low rates of reproduction and natural mortality. Their populations are susceptible to disturbance from human activities, such as the exploration and development of mineral resources or hunting. Polar bear populations have been an important renewable resource available to coastal communities throughout the Arctic for thousands of years.

  5. Polarized rainbow.

    PubMed

    Können, G P; de Boer, J H

    1979-06-15

    The Airy theory of the rainbow is extended to polarized light. For both polarization directions a simple analytic expression is obtained for the intensity distribution as a function of the scattering angle in terms of the Airy function and its derivative. This approach is valid at least down to droplet diameters of 0.3 mm in visible light. The degree of polarization of the rainbow is less than expected from geometrical optics; it increases with droplet size. For a droplet diameter >1 mm the locations of the supernumerary rainbows are equal for both polarization directions, but for a diameter <1 mm the supernumerary rainbows of the weaker polarization component are located between those in the strong component. PMID:20212586

  6. Moller Polarimetry with Atomic Hydrogen Targets

    SciTech Connect

    Eugene Chudakov; Vladimir Luppov

    2003-10-19

    A novel proposal of using polarized atomic hydrogen gas, stored in an ultra-cold magnetic trap, as the target for electron beam polarimetry based on Moller scattering is discussed. Such a target of practically 100% polarized electrons could provide a superb systematic accuracy of about 0.5% for beam polarization measurements. The feasibility studies for the CEBAF electron beam have been performed.

  7. Polar Glaciology

    NASA Technical Reports Server (NTRS)

    Robin, G. D.

    1984-01-01

    Two fields of research on polar ice sheets are likely to be of dominant interest during the 1990s. These are: the role of polar ice sheets in the hydrological cycle ocean-atmosphere-ice sheets-oceans, especially in relation to climate change; and the study and interpretation of material in deep ice cores to provide improved knowledge of past climates and of the varying levels of atmospheric constituents such as CO2, NOx, SO2, aerosols, etc., over the past 200,000 years. Both topics require a better knowledge of ice dynamics. Many of the studies that should be undertaken in polar regions by Earth Observing System require similar instruments and techniques to those used elsewhere over oceans and inland surfaces. However to study polar regions two special requirements need to be met: Earth Observing System satellite(s) need to be in a sufficiently high inclination orbit to cover most of the polar regions. Instruments must also be adapted, often by relatively limited changes, to give satisfactory data over polar ice. The observational requirements for polar ice sheets in the 1990s are summarized.

  8. Real and hybrid atomic orbitals

    NASA Astrophysics Data System (ADS)

    Cook, D. B.; Fowler, P. W.

    1981-09-01

    It is shown that the Schrödinger equation for the hydrogenlike atom separates in both spheroconal and prolate spheroidal coordinates and that these separations provide a sound theoretical basis for the real and hybrid atomic orbitals. Thus the real and hybrid atomic orbitals have as sound a pedigree as the more familiar complex orbitals based on the separation of the Schrödinger equation in spherical polar coordinates.

  9. Scattering Polarization in the Chromosphere

    NASA Technical Reports Server (NTRS)

    Keller, C. U.; Sheeley, N. R., Jr.

    1999-01-01

    Scattering polarization from the photosphere observed close to the solar limb has recently become of interest to study turbulent magnetic fields, abundances, and radiative transfer effects. We extend these studies by measuring the scattering polarization off the limb, i.e. in the chromosphere. However, instrumental effects are much more pronounced and more complicated than those affecting on-disk measurements. In particular, scattered light from the telescope mirrors leads to a new type of instrumental polarization that we describe in detail. The differences between the linearly polarized spectra on the disk and off the limb are often very substantial. Here we show the profiles of HeI D(sub 3), the OI triplet at 777 nm, and the Nal D lines. The change in the latter is in reasonable agreement with the recent modeling efforts of atomic polarization in the lower level by Landi Degl'Innocenti (1998).

  10. Voltage linearity modulation and polarity dependent conduction in metal-insulator-metal capacitors with atomic-layer-deposited Al{sub 2}O{sub 3}/ZrO{sub 2}/SiO{sub 2} nano-stacks

    SciTech Connect

    Zhu, Bao; Liu, Wen-Jun; Wei, Lei; Zhang, David Wei; Jiang, Anquan; Ding, Shi-Jin

    2015-07-07

    Excellent voltage linearity of metal-insulator-metal (MIM) capacitors is highly required for next generation radio frequency integration circuits. In this work, employing atomic layer deposition technique, we demonstrated how the voltage linearity of MIM capacitors was modulated by adding different thickness of SiO{sub 2} layer to the nano-stack of Al{sub 2}O{sub 3}/ZrO{sub 2}. It was found that the quadratic voltage coefficient of capacitance (α) can be effectively reduced from 1279 to −75 ppm/V{sup 2} with increasing the thickness of SiO{sub 2} from zero to 4 nm, which is more powerful than increasing the thickness of ZrO{sub 2} in the Al{sub 2}O{sub 3}/ZrO{sub 2} stack. This is attributed to counteraction between the positive α for Al{sub 2}O{sub 3}/ZrO{sub 2} and the negative one for SiO{sub 2} in the MIM capacitors with Al{sub 2}O{sub 3}/ZrO{sub 2}/SiO{sub 2} stacks. Interestingly, voltage-polarity dependent conduction behaviors in the MIM capacitors were observed. For electron bottom-injection, the addition of SiO{sub 2} obviously suppressed the leakage current; however, it abnormally increased the leakage current for electron top-injection. These are ascribed to the co-existence of shallow and deep traps in ZrO{sub 2}, and the former is in favor of the field-assisted tunnelling conduction and the latter contributes to the trap-assisted tunnelling process. The above findings will be beneficial to device design and process optimization for high performance MIM capacitors.

  11. Voltage linearity modulation and polarity dependent conduction in metal-insulator-metal capacitors with atomic-layer-deposited Al2O3/ZrO2/SiO2 nano-stacks

    NASA Astrophysics Data System (ADS)

    Zhu, Bao; Liu, Wen-Jun; Wei, Lei; Zhang, David Wei; Jiang, Anquan; Ding, Shi-Jin

    2015-07-01

    Excellent voltage linearity of metal-insulator-metal (MIM) capacitors is highly required for next generation radio frequency integration circuits. In this work, employing atomic layer deposition technique, we demonstrated how the voltage linearity of MIM capacitors was modulated by adding different thickness of SiO2 layer to the nano-stack of Al2O3/ZrO2. It was found that the quadratic voltage coefficient of capacitance (α) can be effectively reduced from 1279 to -75 ppm/V2 with increasing the thickness of SiO2 from zero to 4 nm, which is more powerful than increasing the thickness of ZrO2 in the Al2O3/ZrO2 stack. This is attributed to counteraction between the positive α for Al2O3/ZrO2 and the negative one for SiO2 in the MIM capacitors with Al2O3/ZrO2/SiO2 stacks. Interestingly, voltage-polarity dependent conduction behaviors in the MIM capacitors were observed. For electron bottom-injection, the addition of SiO2 obviously suppressed the leakage current; however, it abnormally increased the leakage current for electron top-injection. These are ascribed to the co-existence of shallow and deep traps in ZrO2, and the former is in favor of the field-assisted tunnelling conduction and the latter contributes to the trap-assisted tunnelling process. The above findings will be beneficial to device design and process optimization for high performance MIM capacitors.

  12. Polarizing cues.

    PubMed

    Nicholson, Stephen P

    2012-01-01

    People categorize themselves and others, creating ingroup and outgroup distinctions. In American politics, parties constitute the in- and outgroups, and party leaders hold sway in articulating party positions. A party leader's endorsement of a policy can be persuasive, inducing co-partisans to take the same position. In contrast, a party leader's endorsement may polarize opinion, inducing out-party identifiers to take a contrary position. Using survey experiments from the 2008 presidential election, I examine whether in- and out-party candidate cues—John McCain and Barack Obama—affected partisan opinion. The results indicate that in-party leader cues do not persuade but that out-party leader cues polarize. This finding holds in an experiment featuring President Bush in which his endorsement did not persuade Republicans but it polarized Democrats. Lastly, I compare the effect of party leader cues to party label cues. The results suggest that politicians, not parties, function as polarizing cues. PMID:22400143

  13. Nuclear reactivity control using laser induced polarization

    DOEpatents

    Bowman, Charles D.

    1991-01-01

    A control element for reactivity control of a fission source provides an atomic density of .sup.3 He in a control volume which is effective to control criticality as the .sup.3 He is spin-polarized. Spin-polarization of the .sup.3 He affects the cross section of the control volume for fission neutrons and hence, the reactivity. An irradiation source is directed within the .sup.3 He for spin-polarizing the .sup.3 He. An alkali-metal vapor may be included with the .sup.3 He where a laser spin-polarizes the alkali-metal atoms which in turn, spin-couple with .sup.3 He to spin-polarize the .sup.3 He atoms.

  14. Nuclear reactivity control using laser induced polarization

    DOEpatents

    Bowman, Charles D.

    1990-01-01

    A control element for reactivity control of a fission source provides an atomic density of .sup.3 He in a control volume which is effective to control criticality as the .sup.3 He is spin-polarized. Spin-polarization of the .sup.3 He affects the cross section of the control volume for fission neturons and hence, the reactivity. An irradiation source is directed within the .sup.3 He for spin-polarizing the .sup.3 He. An alkali-metal vapor may be included with the .sup.3 He where a laser spin-polarizes the alkali-metal atoms which in turn, spin-couple with .sup.3 He to spin-polarize the .sup.3 He atoms.

  15. Polar motion

    NASA Technical Reports Server (NTRS)

    Kolenkiewicz, R.

    1973-01-01

    Tracking of the Beacon Explorer-C satellite by a precision laser system was used to measure the polar motion and solid earth tide. The tidal perturbation of satellite latitude is plotted as variation in maximum latitude in seconds of arc on earth's surface as a function of the date, and polar motion is shown by plotting the variation in latitude of the laser in seconds of arc along the earth's surface as a function of date

  16. Understanding ultracold polar molecules

    NASA Astrophysics Data System (ADS)

    Julienne, Paul

    2009-05-01

    The successful production of a dense sample of ultracold ground state KRb polar molecules [1] opens the door to a new era of research with dipolar gases and lattices of such species. This feat was achieved by first associating a K and a Rb atom to make a weakly bound Feshbach molecule and then coherently transferring the population to the ground vibrational level of the molecule. This talk focuses on theoretical issues associated with making and using ultracold polar molecules, using KRb as an example [2]. Full understanding of this species and the processes by which it is made requires taking advantage of accurate molecular potentials [3], ab initio calculations [4], and the properties of the long-range potential. A highly accurate model is available for KRb for all bound states below the ground state separated atom limit and could be constructed for other species. The next step is to develop an understanding of the interactions between polar molecules, and their control in the ultracold domain. Understanding long-range interactions and threshold resonances will be crucial for future work. [1] K.-K. Ni, et al, Science 322, 231(2008). [2] P. S. Julienne, arXiv:0812:1233. [3] Pashov et al., Phys. Rev. A76, 022511 (2007). [4] S. Kotochigova, et al., arXiv:0901.1486.

  17. Laser-induced photofragmentation of triethylaluminum: Modeling H-atom production

    NASA Astrophysics Data System (ADS)

    Brum, Jeffrey L.; Deshmukh, Subhash; Koplitz, Brent

    1990-12-01

    A rate-equation approach is presented that models H-atom formation during the pulsed laser photolysis of a triethyl metal compound, the specific case being triethylaluminum excited at 193 nm. An excimer laser initiates the chemistry under collisionless conditions, and H atoms are produced that are detected using two-photon (121.6+364.7 nm) ionization. Experimentally, the H-atom intensity is monitored as a function of photolysis laser power. Mechanistically, the primary photodissociation step is postulated to involve cleavage of the metal-carbon bond, thereby producing an ethyl radical. This species can then either: (1) form C2H4 and H directly; or (2) absorb an additional photon and produce an H-atom photofragment. The rate equations and their solutions allow one to calculate how H-atom production should vary as a function of photolysis laser power, and the interplay between the two H-atom production channels is calculated for various absorption cross sections and dissociation rates. A comparison with experimental power dependence data suggests that an overall one-photon dissociation process predominates under the experimental conditions actually used.

  18. Chiral atomically thin films

    NASA Astrophysics Data System (ADS)

    Kim, Cheol-Joo; Sánchez-Castillo, A.; Ziegler, Zack; Ogawa, Yui; Noguez, Cecilia; Park, Jiwoong

    2016-06-01

    Chiral materials possess left- and right-handed counterparts linked by mirror symmetry. These materials are useful for advanced applications in polarization optics, stereochemistry and spintronics. In particular, the realization of spatially uniform chiral films with atomic-scale control of their handedness could provide a powerful means for developing nanodevices with novel chiral properties. However, previous approaches based on natural or grown films, or arrays of fabricated building blocks, could not offer a direct means to program intrinsic chiral properties of the film on the atomic scale. Here, we report a chiral stacking approach, where two-dimensional materials are positioned layer-by-layer with precise control of the interlayer rotation (θ) and polarity, resulting in tunable chiral properties of the final stack. Using this method, we produce left- and right-handed bilayer graphene, that is, a two-atom-thick chiral film. The film displays one of the highest intrinsic ellipticity values (6.5 deg μm–1) ever reported, and a remarkably strong circular dichroism (CD) with the peak energy and sign tuned by θ and polarity. We show that these chiral properties originate from the large in-plane magnetic moment associated with the interlayer optical transition. Furthermore, we show that we can program the chiral properties of atomically thin films layer-by-layer by producing three-layer graphene films with structurally controlled CD spectra.

  19. Chiral atomically thin films.

    PubMed

    Kim, Cheol-Joo; Sánchez-Castillo, A; Ziegler, Zack; Ogawa, Yui; Noguez, Cecilia; Park, Jiwoong

    2016-06-01

    Chiral materials possess left- and right-handed counterparts linked by mirror symmetry. These materials are useful for advanced applications in polarization optics, stereochemistry and spintronics. In particular, the realization of spatially uniform chiral films with atomic-scale control of their handedness could provide a powerful means for developing nanodevices with novel chiral properties. However, previous approaches based on natural or grown films, or arrays of fabricated building blocks, could not offer a direct means to program intrinsic chiral properties of the film on the atomic scale. Here, we report a chiral stacking approach, where two-dimensional materials are positioned layer-by-layer with precise control of the interlayer rotation (θ) and polarity, resulting in tunable chiral properties of the final stack. Using this method, we produce left- and right-handed bilayer graphene, that is, a two-atom-thick chiral film. The film displays one of the highest intrinsic ellipticity values (6.5 deg μm(-1)) ever reported, and a remarkably strong circular dichroism (CD) with the peak energy and sign tuned by θ and polarity. We show that these chiral properties originate from the large in-plane magnetic moment associated with the interlayer optical transition. Furthermore, we show that we can program the chiral properties of atomically thin films layer-by-layer by producing three-layer graphene films with structurally controlled CD spectra. PMID:26900756

  20. Creation of polarization gradients from superposition of counter propagating vector LG beams.

    PubMed

    Vyas, Sunil; Kozawa, Yuichi; Miyamoto, Yoko

    2015-12-28

    We present a detailed theoretical analysis of the formation of standing waves using cylindrically polarized vector Laguerre-Gaussian (LG) beams. It is shown that complex interplay between the radial and azimuthal polarization state can be used to realize different kinds of polarization gradients with cylindrically symmetric polarization distribution. Expressions for four different cases are presented and local dynamics of spatial polarization distribution is studied. We show cylindrically symmetric Sisyphus and corkscrew type polarization gradients can be obtained from vector LG beams. The optical landscape presented here with spatially periodic polarization patterns may find important applications in the field of atom optics, atom interferometry, atom lithography, and optical trapping. PMID:26832055

  1. VCSELs for atomic clocks

    NASA Astrophysics Data System (ADS)

    Serkland, Darwin K.; Peake, Gregory M.; Geib, Kent M.; Lutwak, Robert; Garvey, R. Michael; Varghese, Mathew; Mescher, Mark

    2006-02-01

    The spectroscopic technique of coherent population trapping (CPT) enables an all-optical interrogation of the groundstate hyperfine splitting of cesium (or rubidium), compared to the optical-microwave double resonance technique conventionally employed in atomic frequency standards. All-optical interrogation enables the reduction of the size and power consumption of an atomic clock by two orders of magnitude, and vertical-cavity surface-emitting lasers (VCSELs) are preferred optical sources due to their low power consumption and circular output beam. Several research teams are currently using VCSELs for DARPA's chip-scale atomic clock (CSAC) program with the goal of producing an atomic clock having a volume < 1 cm^3, a power consumption < 30 mW, and an instability (Allan deviation) < 1x10^-11 during a 1-hour averaging interval. This paper describes the VCSEL requirements for CPT-based atomic clocks, which include single mode operation, single polarization operation, modulation bandwidth > 4 GHz, low power consumption (for the CSAC), narrow linewidth, and low relative intensity noise (RIN). A significant manufacturing challenge is to reproducibly obtain the required wavelength at the specified VCSEL operating temperature and drive current. Data are presented that show the advantage of operating at the D1 (rather than D2) resonance of the alkali atoms. Measurements of VCSEL linewidth will be discussed in particular, since atomic clock performance is especially sensitive to this parameter.

  2. Ion-Atom Cold Collisions and Atomic Clocks

    NASA Technical Reports Server (NTRS)

    Prestage, John D.; Maleki, Lute; Tjoelker, Robert L.

    1997-01-01

    Collisions between ultracold neutral atoms have for some time been the subject of investigation, initially with hydrogen and more recently with laser cooled alkali atoms. Advances in laser cooling and trapping of neutral atoms in a Magneto-Optic Trap (MOT) have made cold atoms available as the starting point for many laser cooled atomic physics investigations. The most spectacularly successful of these, the observation of Bose-Einstein Condensation (BEC) in a dilute ultra-cold spin polarized atomic vapor, has accelerated the study of cold collisions. Experimental and theoretical studies of BEC and the long range interaction between cold alkali atoms is at the boundary of atomic and low temperature physics. Such studies have been difficult and would not have been possible without the development and advancement of laser cooling and trapping of neutral atoms. By contrast, ion-atom interactions at low temperature, also very difficult to study prior to modern day laser cooling, have remained largely unexplored. But now, many laboratories worldwide have almost routine access to cold neutral atoms. The combined technologies of ion trapping, together with laser cooling of neutrals has made these studies experimentally feasible and several very important, novel applications might come out of such investigations . This paper is an investigation of ion-atom interactions in the cold and ultra-cold temperature regime. Some of the collisional ion-atom interactions present at room temperature are very much reduced in the low temperature regime. Reaction rates for charge transfer between unlike atoms, A + B(+) approaches A(+) + B, are expected to fall rapidly with temperature, approximately as T(sup 5/2). Thus, cold mixtures of atoms and ions are expected to coexist for very long times, unlike room temperature mixtures of the same ion-atom combination. Thus, it seems feasible to cool ions via collisions with laser cooled atoms. Many of the conventional collisional interactions

  3. Liquid atomization

    NASA Astrophysics Data System (ADS)

    Bayvel, L.; Orzechowski, Z.

    The present text defines the physical processes of liquid atomization, the primary types of atomizers and their design, and ways of measuring spray characteristics; it also presents experimental investigation results on atomizers and illustrative applications for them. Attention is given to the macrostructural and microstructural parameters of atomized liquids; swirl, pneumatic, and rotary atomizers; and optical drop sizing methods, with emphasis on nonintrusive optical methods.

  4. Polar Stratigraphy

    NASA Technical Reports Server (NTRS)

    1999-01-01

    These three images were taken on three different orbits over the north polar cap in April 1999. Each shows a different part of the same ice-free trough. The left and right images are separated by a distance of more than 100 kilometers (62 miles). Note the similar layers in each image.

  5. Political polarization

    PubMed Central

    Dixit, Avinash K.; Weibull, Jörgen W.

    2007-01-01

    Failures of government policies often provoke opposite reactions from citizens; some call for a reversal of the policy, whereas others favor its continuation in stronger form. We offer an explanation of such polarization, based on a natural bimodality of preferences in political and economic contexts and consistent with Bayesian rationality. PMID:17452633

  6. Polarization properties of the “photon pistol”

    NASA Astrophysics Data System (ADS)

    Reshetov, V. A.

    2012-10-01

    The deterministic single-photon emission by means of STIRAP through the atoms with degenerate levels is studied. The expression for the polarization matrix of the emitted photon is obtained and its dependence on the polarization of the driving laser field and on the initial atomic state is examined.

  7. The physics of polarization

    NASA Astrophysics Data System (ADS)

    Landi Degl'Innocenti, Egidio

    ). Finally, the third part (Sects. 15-19) is devoted to give a sketch of the theory of the generation and transfer of polarized radiation in spectral lines. After a general introduction to the argument (Sect. 15), the concepts of density-matrix and of atomic polarization are illustrated in Sect. 16. In Sect. 17, a parallelism is established, within the framework of the theory of stellar atmospheres, between the usual formalism, which neglects polarization phenomena, and the more involved formalism needed for the interpretation of spectro-polarimetric observations. Some consequences of the radiative transfer equations for polarized radiation, pointing to the importance of dichroism phenomena in establishing the amplification condition via stimulated emission, are discussed in Sect. 18. The last section (Sect. 19) is devoted to introduce the problem of finding a self-consistent solution of the radiative transfer equations for polarized radiation and of the statistical equilibrium equations for the density matrix (non-LTE of the 2nd kind).

  8. Surface spin polarization induced ferromagnetic Ag nanoparticles

    NASA Astrophysics Data System (ADS)

    Shih, Po-Hsun; Li, Wen-Hsien; Wu, Sheng Yun

    2016-05-01

    We report on the observation of ferromagnetic spin polarized moments in 4.5 nm Ag nanoparticles. Both ferromagnetic and diamagnetic responses to an applied magnetic field were detected. The spin polarized moments shown under non-linear thermoinduced magnetization appeared on the surface atoms, rather than on all the atoms in particles. The saturation magnetization departed substantially from the Bloch T3/2-law, showing the existence of magnetic anisotropy. The Heisenberg ferromagnetic spin wave model for Ha-aligned moments was then employed to identify the magnetic anisotropic energy gap of ~0.12 meV. Our results may be understood by assuming the surface magnetism model, in which the surface atoms give rise to polarized moments while the core atoms produce diamagnetic responses.

  9. Polar metals by geometric design

    NASA Astrophysics Data System (ADS)

    Kim, T. H.; Puggioni, D.; Yuan, Y.; Xie, L.; Zhou, H.; Campbell, N.; Ryan, P. J.; Choi, Y.; Kim, J.-W.; Patzner, J. R.; Ryu, S.; Podkaminer, J. P.; Irwin, J.; Ma, Y.; Fennie, C. J.; Rzchowski, M. S.; Pan, X. Q.; Gopalan, V.; Rondinelli, J. M.; Eom, C. B.

    2016-05-01

    Gauss’s law dictates that the net electric field inside a conductor in electrostatic equilibrium is zero by effective charge screening; free carriers within a metal eliminate internal dipoles that may arise owing to asymmetric charge distributions. Quantum physics supports this view, demonstrating that delocalized electrons make a static macroscopic polarization, an ill-defined quantity in metals—it is exceedingly unusual to find a polar metal that exhibits long-range ordered dipoles owing to cooperative atomic displacements aligned from dipolar interactions as in insulating phases. Here we describe the quantum mechanical design and experimental realization of room-temperature polar metals in thin-film ANiO3 perovskite nickelates using a strategy based on atomic-scale control of inversion-preserving (centric) displacements. We predict with ab initio calculations that cooperative polar A cation displacements are geometrically stabilized with a non-equilibrium amplitude and tilt pattern of the corner-connected NiO6 octahedra—the structural signatures of perovskites—owing to geometric constraints imposed by the underlying substrate. Heteroepitaxial thin-films grown on LaAlO3 (111) substrates fulfil the design principles. We achieve both a conducting polar monoclinic oxide that is inaccessible in compositionally identical films grown on (001) substrates, and observe a hidden, previously unreported, non-equilibrium structure in thin-film geometries. We expect that the geometric stabilization approach will provide novel avenues for realizing new multifunctional materials with unusual coexisting properties.

  10. Cell polarity

    PubMed Central

    Romereim, Sarah M

    2011-01-01

    Despite extensive genetic analysis of the dynamic multi-phase process that transforms a small population of lateral plate mesoderm into the mature limb skeleton, the mechanisms by which signaling pathways regulate cellular behaviors to generate morphogenetic forces are not known. Recently, a series of papers have offered the intriguing possibility that regulated cell polarity fine-tunes the morphogenetic process via orienting cell axes, division planes and cell movements. Wnt5a-mediated non-canonical signaling, which may include planar cell polarity, has emerged as a common thread in the otherwise distinct signaling networks that regulate morphogenesis in each phase of limb development. These findings position the limb as a key model to elucidate how global tissue patterning pathways direct local differences in cell behavior that, in turn, generate growth and form. PMID:22064549

  11. Polarization Labeling Spectroscopy of Hollow Lithium

    NASA Astrophysics Data System (ADS)

    Huang, M.-T.; Wehlitz, R.; Cherepkov, N. A.; Azuma, Y.; Depaola, B. D.; Nagata, T.; Hasegawa, S.; Levin, J. C.; Sellin, I. A.

    1998-05-01

    Utilization of polarized or aligned targets can provide valuable information on atomic photoionization and excitation processes. (M. Meyer et al.), Phys. Rev. Lett. 59, 2963 (1987) We measured numerous even-parity doubly core excited ``hollow lithium'' resonances using monchromatized synchrotron radiation derived from an undulator, and laser excited lithium targets. The excited 1s^22p ^2Po targets, were aligned or polarized by laser pumping, and measurements were made with various combinations with the polarization of synchrotron radiation. The intensity pattern of the photoion spectrum shows clear polarization dependence and provides useful clues to the analysis.

  12. Collisional pumping in polarized sodium vapor

    SciTech Connect

    Kaplan, S.N.; pyle, R.V.; Ruby, L.; Schlachter, A.S.; Stearns, J.W.; Anderson, L.W.

    1986-01-01

    Collisional pumping has been proposed as a mechanism for efficient transfer of spin from an electron-spin-polarized target to the nuclei of a fast atom or ion beam. Collisional pumping takes place in low magnetic fields, can give polarization transfer approaching 100%, and offers the potential for producing polarized beams orders of magnitude more intense than presently achieved. Recently reported calculations of electronic spin-exchange cross sections at useful ion-source energies suggest significantly greater rates of pumping than first estimated, and give cause for increased optimism about sucessful implementation. Collisional pumping is described, and beam characteristics are given for prototype polarized source parameters.

  13. Birefringence lens effects of an atom ensemble enhanced by an electromagnetically induced transparency

    SciTech Connect

    Zhang, H. R.; Sun, C. P.; Zhou Lan

    2009-07-15

    We study the optical control for birefringence of a polarized light by an atomic ensemble with a tripod configuration, which is mediated by the electromagnetically induced transparency with a spatially inhomogeneous laser. The atomic ensemble splits the linearly polarized light ray into two orthogonally polarized components, whose polarizations depend on quantum superposition of the initial states of the atomic ensemble. Accompanied with this splitting, the atomic ensemble behaves as a birefringent lens, which allows one polarized light ray passing through straightly while focuses the other light of vertical polarization with finite aberration of focus.

  14. Polar Textures

    NASA Technical Reports Server (NTRS)

    2005-01-01

    [figure removed for brevity, see original site] Context image for PIA03646 Polar Textures

    This VIS image shows part of the south polar region. The ejecta from the relatively young crater covers the rougher textured polar surface.

    Image information: VIS instrument. Latitude 81S, Longitude 54.5E. 17 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with Project policies at a later time.

    NASA's Jet Propulsion Laboratory manages the 2001 Mars Odyssey mission for NASA's Office of Space Science, Washington, D.C. The Thermal Emission Imaging System (THEMIS) was developed by Arizona State University, Tempe, in collaboration with Raytheon Santa Barbara Remote Sensing. The THEMIS investigation is led by Dr. Philip Christensen at Arizona State University. Lockheed Martin Astronautics, Denver, is the prime contractor for the Odyssey project, and developed and built the orbiter. Mission operations are conducted jointly from Lockheed Martin and from JPL, a division of the California Institute of Technology in Pasadena.

  15. Entanglement of remote atomic qubits.

    PubMed

    Matsukevich, D N; Chanelière, T; Jenkins, S D; Lan, S-Y; Kennedy, T A B; Kuzmich, A

    2006-01-27

    We report observations of entanglement of two remote atomic qubits, achieved by generating an entangled state of an atomic qubit and a single photon at site , transmitting the photon to site in an adjacent laboratory through an optical fiber, and converting the photon into an atomic qubit. Entanglement of the two remote atomic qubits is inferred by performing, locally, quantum state transfer of each of the atomic qubits onto a photonic qubit and subsequent measurement of polarization correlations in violation of the Bell inequality [EQUATION: SEE TEXT]. We experimentally determine [EQUATION: SEE TEXT]. Entanglement of two remote atomic qubits, each qubit consisting of two independent spin wave excitations, and reversible, coherent transfer of entanglement between matter and light represent important advances in quantum information science. PMID:16486672

  16. POLARIZED HYDROGEN JET TARGET FOR MEASUREMENT OF RHIC PROTON BEAM POLARIZATION.

    SciTech Connect

    MAKDISI,Y.; WISE,T.; CHAPMAN,M.; GRAHAM,D.; KPONOU,A.; MAHLER,G.; MENG,W.; NASS,A.; RITTER,J.

    2005-01-28

    The performance and unique features of the RHIC polarized jet target and our solutions to the important design constraints imposed on the jet by the RHIC environment are described. The target polarization and thickness were measured to be 0.924 {+-} 2% and 1.3 {+-} 0.2 x 10{sup 12} atoms/cm{sup 2} respectively.

  17. Coherent population trapping with polarization modulation

    NASA Astrophysics Data System (ADS)

    Yun, Peter; Guérandel, Stéphane; de Clercq, Emeric

    2016-06-01

    Coherent population trapping (CPT) is extensively studied for future vapor cell clocks of high frequency stability. In the constructive polarization modulation CPT scheme, a bichromatic laser field with polarization and phase synchronously modulated is applied on an atomic medium. A high contrast CPT signal is observed in this so-called double-modulation configuration, due to the fact that the atomic population does not leak to the extreme Zeeman states, and that the two CPT dark states, which are produced successively by the alternate polarizations, add constructively. Here, we experimentally investigate CPT signal dynamics first in the usual configuration, a single circular polarization. The double-modulation scheme is then addressed in both cases: one pulse Rabi interaction and two pulses Ramsey interaction. The impact and the optimization of the experimental parameters involved in the time sequence are reviewed. We show that a simple seven-level model explains the experimental observations. The double-modulation scheme yields a high contrast similar to the one of other high contrast configurations like push-pull optical pumping or crossed linear polarization scheme, with a setup allowing a higher compactness. The constructive polarization modulation is attractive for atomic clock, atomic magnetometer, and high precision spectroscopy applications.

  18. Epitaxial growth of polar KTaO3 thin-films on polar perovskite substrates

    NASA Astrophysics Data System (ADS)

    Thompson, J.; Nichols, J.; Hwang, J.; Seo, S. S. A.

    2014-03-01

    The atomic polarity plays an important role in a wide range of physical phenomena at heterointerfaces. For example, the polar/non-polar nature of a LaAlO3/SrTiO3 system induces partial conducting electrons at the heterointerfaces to avoid diverging electrostatic potential, the so-called ``polar catastrophe,'' which results in intriguing two-dimensional transport and magnetic properties. In this presentation, we discuss another system in which the role of the polar interface is important: the KTaO3/GdScO3 (KTO/GSO) polar/polar system. At the KTO/GSO interface, there is a ``polar conflict'' heterointerface along the [001] direction, where the AO and BO2 layers have reversed net charges so that there is a conflict between the chemical bonding and the electrostatic charges, i.e. K1+O2-(1-)/Sc3+O24- (1-) or Ta5+O24- (1 +) /Gd3+O2-(1 +) , which is unstable in the electrostatic point of view. We ask a fundamental question: ``How is the polar conflict resolved in the atomically flat heterointerfaces of such polar/polar systems?'' We have synthesized epitaxial KTO thin films on GSO substrates using pulsed laser deposition. From X-ray diffraction and high-resolution transmission electron microscopy, we have observed that the polar conflict is quite effectively avoided by forming only two non-polar mono-layers at the heterointerface, resulting in high-quality epitaxial thin films on top of the layers. Our result suggests a new way to create two-dimensional confined layers using the polar conflict of the heterointerfaces of two polar materials.

  19. Polar Landforms

    NASA Technical Reports Server (NTRS)

    2005-01-01

    10 August 2005 This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) image shows eroded remnants of carbon dioxide ice in the south polar residual cap of Mars. The scarps that outline each small mesa have retreated about 3 meters (10 feet) per Mars year since MGS began orbiting the red planet in 1997.

    Location near: 87.0oS, 31.9oW Image width: width: 3 km (1.9 mi) Illumination from: upper left Season: Southern Spring

  20. Polar ozone

    NASA Technical Reports Server (NTRS)

    Solomon, S.; Grose, W. L.; Jones, R. L.; Mccormick, M. P.; Molina, Mario J.; Oneill, A.; Poole, L. R.; Shine, K. P.; Plumb, R. A.; Pope, V.

    1990-01-01

    The observation and interpretation of a large, unexpected ozone depletion over Antarctica has changed the international scientific view of stratospheric chemistry. The observations which show the veracity, seasonal nature, and vertical structure of the Antarctic ozone hole are presented. Evidence for Arctic and midlatitude ozone loss is also discussed. The chemical theory for Antarctic ozone depletion centers around the occurrence of polar stratospheric clouds (PSCs) in Antarctic winter and spring; the climatology and radiative properties of these clouds are presented. Lab studies of the physical properties of PSCs and the chemical processes that subsequently influence ozone depletion are discussed. Observations and interpretation of the chemical composition of the Antarctic stratosphere are described. It is shown that the observed, greatly enhanced abundances of chlorine monoxide in the lower stratosphere are sufficient to explain much if not all of the ozone decrease. The dynamic meteorology of both polar regions is given, interannual and interhemispheric variations in dynamical processes are outlined, and their likely roles in ozone loss are discussed.

  1. Polar Markings

    NASA Technical Reports Server (NTRS)

    2006-01-01

    [figure removed for brevity, see original site] Context image for PIA02155 Polar Markings

    These bright and dark markings occurred near the end of summer in the south polar region. The dark material is likely dust that has been freed of frost cover.

    Image information: VIS instrument. Latitude -76.3N, Longitude 84.9E. 17 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with Project policies at a later time.

    NASA's Jet Propulsion Laboratory manages the 2001 Mars Odyssey mission for NASA's Office of Space Science, Washington, D.C. The Thermal Emission Imaging System (THEMIS) was developed by Arizona State University, Tempe, in collaboration with Raytheon Santa Barbara Remote Sensing. The THEMIS investigation is led by Dr. Philip Christensen at Arizona State University. Lockheed Martin Astronautics, Denver, is the prime contractor for the Odyssey project, and developed and built the orbiter. Mission operations are conducted jointly from Lockheed Martin and from JPL, a division of the California Institute of Technology in Pasadena.

  2. Polar Layers

    NASA Technical Reports Server (NTRS)

    2006-01-01

    [figure removed for brevity, see original site] Context image for PIA02153 Polar Layers

    This image of the south polar region shows layered material. It is not known if the layers are formed yearly or if they form over the period of 10s to 100s of years or more.

    Image information: VIS instrument. Latitude -80.3N, Longitude 296.2E. 17 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with Project policies at a later time.

    NASA's Jet Propulsion Laboratory manages the 2001 Mars Odyssey mission for NASA's Office of Space Science, Washington, D.C. The Thermal Emission Imaging System (THEMIS) was developed by Arizona State University, Tempe, in collaboration with Raytheon Santa Barbara Remote Sensing. The THEMIS investigation is led by Dr. Philip Christensen at Arizona State University. Lockheed Martin Astronautics, Denver, is the prime contractor for the Odyssey project, and developed and built the orbiter. Mission operations are conducted jointly from Lockheed Martin and from JPL, a division of the California Institute of Technology in Pasadena.

  3. Polar Ridges

    NASA Technical Reports Server (NTRS)

    2006-01-01

    [figure removed for brevity, see original site] Context image for PIA03662 Polar Ridges

    This ridge system is located in the south polar region.

    Image information: VIS instrument. Latitude -81.7N, Longitude 296.5E. 17 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with Project policies at a later time.

    NASA's Jet Propulsion Laboratory manages the 2001 Mars Odyssey mission for NASA's Office of Space Science, Washington, D.C. The Thermal Emission Imaging System (THEMIS) was developed by Arizona State University, Tempe, in collaboration with Raytheon Santa Barbara Remote Sensing. The THEMIS investigation is led by Dr. Philip Christensen at Arizona State University. Lockheed Martin Astronautics, Denver, is the prime contractor for the Odyssey project, and developed and built the orbiter. Mission operations are conducted jointly from Lockheed Martin and from JPL, a division of the California Institute of Technology in Pasadena.

  4. Polar Textures

    NASA Technical Reports Server (NTRS)

    2005-01-01

    [figure removed for brevity, see original site] Context image for PIA03638 Polar Textures

    This image illustrates the variety of textures that appear in the south polar region during late summer.

    Image information: VIS instrument. Latitude 80.5S, Longitude 57.9E. 17 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with Project policies at a later time.

    NASA's Jet Propulsion Laboratory manages the 2001 Mars Odyssey mission for NASA's Office of Space Science, Washington, D.C. The Thermal Emission Imaging System (THEMIS) was developed by Arizona State University, Tempe, in collaboration with Raytheon Santa Barbara Remote Sensing. The THEMIS investigation is led by Dr. Philip Christensen at Arizona State University. Lockheed Martin Astronautics, Denver, is the prime contractor for the Odyssey project, and developed and built the orbiter. Mission operations are conducted jointly from Lockheed Martin and from JPL, a division of the California Institute of Technology in Pasadena.

  5. Polar Terrains

    NASA Technical Reports Server (NTRS)

    2005-01-01

    [figure removed for brevity, see original site] Context image for PIA03577 Polar Terrains

    The region surrounding the South Polar Cap contains many different terrain types. This image shows both etched terrain and a region of 'mounds'.

    Image information: VIS instrument. Latitude 75S, Longitude 286.5E. 17 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with Project policies at a later time.

    NASA's Jet Propulsion Laboratory manages the 2001 Mars Odyssey mission for NASA's Office of Space Science, Washington, D.C. The Thermal Emission Imaging System (THEMIS) was developed by Arizona State University, Tempe, in collaboration with Raytheon Santa Barbara Remote Sensing. The THEMIS investigation is led by Dr. Philip Christensen at Arizona State University. Lockheed Martin Astronautics, Denver, is the prime contractor for the Odyssey project, and developed and built the orbiter. Mission operations are conducted jointly from Lockheed Martin and from JPL, a division of the California Institute of Technology in Pasadena.

  6. A method to polarize stored antiprotons to a high degree.

    PubMed

    Rathmann, F; Lenisa, P; Steffens, E; Contalbrigo, M; Dalpiaz, P F; Kacharava, A; Lehrach, A; Lorentz, B; Maier, R; Prasuhn, D; Ströher, H

    2005-01-14

    Polarized antiprotons can be produced in a storage ring by spin-dependent interaction in a purely electron-polarized hydrogen gas target. The polarizing process is based on spin transfer from the polarized electrons of the target atoms to the orbiting antiprotons. After spin filtering for about two beam lifetimes at energies T approximately equal 40-170 MeV using a dedicated large acceptance ring, the antiproton beam polarization would reach P=0.2-0.4. Polarized antiprotons would open new and unique research opportunities for spin-physics experiments in p(-) p interactions. PMID:15698088

  7. Polar Barchans

    NASA Technical Reports Server (NTRS)

    2004-01-01

    20 July 2004 This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) image shows dark, barchan sand dunes of the north polar region of Mars. Barchan dunes are simple, rounded forms with two horns that extend downwind. Inequalities in local wind patterns may result in one horn being extended farther than the other, as is the case for several dunes in this image. The image also shows several barchans may merge to form a long dune ridge. The horns and attendant slip faces on these dunes indicate wind transport of sand from the upper left toward the lower right. The image is located near 77.6oN, 103.6oW. The picture covers an area about 3 km (1.9 mi) wide; sunlight illuminates the scene from the lower left.

  8. Polar Polygons

    NASA Technical Reports Server (NTRS)

    2004-01-01

    26 December 2003 This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) picture displays polygons outlined by cracks in the martian south polar region. This southern summer view was acquired in October 2003 and is located near 86.9oS, 170.6oW. Polygons similar in size and shape to these are common in the arctic and antarctic regions of Earth. On Earth, they indicate the presence (or the past presence) of ground ice and the freeze-thaw cycles that accompany this ice. On Mars, whether ground ice was responsible for these landforms is uncertain, but their presence is suggestive that ground ice may exist or may once have existed in this region. The picture covers an area 3 km (1.9 mi) wide. Sunlight illuminates the scene from the upper left.

  9. Polarized tritium target development

    SciTech Connect

    Jones, C.E.; Fedchak, J.A.; Kowalczyk, R.S.

    1995-08-01

    Work began on the development of a completely sealed polarized tritium target for experiments at CEBAF. Because of the similarities between optical pumping of tritium and hydrogen, all prototype work is done with hydrogen. We constructed a test station for filling glassware with hydrogen, where we can dissociate molecular hydrogen and monitor the purity of the gas. A simple two-cell glass system was constructed, consisting of a region in which the molecular hydrogen is dissociated with an RF discharge and a region where the atoms can be optically pumped. So far, a clean discharge was obtained in the glassware. With this system, we plan to investigate ways to eliminate the discharge from the optical pumping region and test the quality of the discharge once the pumping cell is coated with drifilm.

  10. Photonic multiqubit states from a single atom

    SciTech Connect

    Li Ying; Aolita, Leandro; Kwek, L. C.

    2011-03-15

    We propose a protocol for the creation of photonic Greenberger-Horne-Zeilinger and linear cluster states emitted from a single atom--or ion--coupled to an optical cavity field. The method is based on laser pulses with different polarizations and exploits the atomic transition amplitudes to state-selectively achieve the desired transitions. The scheme lies within reach of current technology.

  11. Atomic supersymmetry

    NASA Technical Reports Server (NTRS)

    Kostelecky, V. Alan

    1993-01-01

    Atomic supersymmetry is a quantum-mechanical supersymmetry connecting the properties of different atoms and ions. A short description of some established results in the subject are provided and a few recent developments are discussed including the extension to parabolic coordinates and the calculation of Stark maps using supersymmetry-based models.

  12. Atomic Calligraphy

    NASA Astrophysics Data System (ADS)

    Imboden, Matthias; Pardo, Flavio; Bolle, Cristian; Han, Han; Tareen, Ammar; Chang, Jackson; Christopher, Jason; Corman, Benjamin; Bishop, David

    2013-03-01

    Here we present a MEMS based method to fabricate devices with a small number of atoms. In standard semiconductor fabrication, a large amount of material is deposited, after which etching removes what is not wanted. This technique breaks down for structures that approach the single atom limit, as it is inconceivable to etch away all but one atom. What is needed is a bottom up method with single or near single atom precision. We demonstrate a MEMS device that enables nanometer position controlled deposition of gold atoms. A digitally driven plate is swept as a flux of gold atoms passes through an aperture. Appling voltages on four comb capacitors connected to the central plate by tethers enable nanometer lateral precision in the xy plane over 15x15 sq. microns. Typical MEMS structures have manufacturing resolutions on the order of a micron. Using a FIB it is possible to mill apertures as small as 10 nm in diameter. Assuming a low incident atomic flux, as well as an integrated MEMS based shutter with microsecond response time, it becomes possible to deposit single atoms. Due to their small size and low power consumption, such nano-printers can be mounted directly in a cryogenic system at ultrahigh vacuum to deposit clean quench condensed metallic structures.

  13. Production and Trapping of Ultracold Polar Molecules

    SciTech Connect

    David, DeMille

    2015-04-21

    We report a set of experiments aimed at the production and trapping of ultracold polar molecules. We begin with samples of laser-cooled and trapped Rb and Cs atoms, and bind them together to form polar RbCs molecules. The binding is accomplished via photoassociation, which uses a laser to catalyze the sticking process. We report results from investigation of a new pathway for photoassociation that can produce molecules in their absolute ground state of vibrational and rotational motion. We also report preliminary observations of collisions between these ground-state molecules and co-trapped atoms.

  14. Liquid atomization

    SciTech Connect

    Walzel, P. )

    1993-01-01

    A systematic review of different liquid atomizers is presented, accompanied by a discussion of various mechanisms of droplet formation in a gas atmosphere as a function of the liquid flow-regime and the geometry of the atomizer. Equations are presented for the calculation of the mean droplet-diameter. In many applications, details of the droplet size distribution are, also, important, e.g., approximate values of the breadth of the droplet formation are given. The efficiency of utilization of mechanical energy in droplet formation is indicated for the different types of atomizers. Atomization is used, in particular, for the following purposes: (1) atomization of fuels; (2) making granular products; (3) carrying out mass-transfer operations; and (4) coating of surfaces.

  15. Cavity enhanced atomic magnetometry

    PubMed Central

    Crepaz, Herbert; Ley, Li Yuan; Dumke, Rainer

    2015-01-01

    Atom sensing based on Faraday rotation is an indispensable method for precision measurements, universally suitable for both hot and cold atomic systems. Here we demonstrate an all-optical magnetometer where the optical cell for Faraday rotation spectroscopy is augmented with a low finesse cavity. Unlike in previous experiments, where specifically designed multipass cells had been employed, our scheme allows to use conventional, spherical vapour cells. Spherical shaped cells have the advantage that they can be effectively coated inside with a spin relaxation suppressing layer providing long spin coherence times without addition of a buffer gas. Cavity enhancement shows in an increase in optical polarization rotation and sensitivity compared to single-pass configurations. PMID:26481853

  16. Cavity enhanced atomic magnetometry.

    PubMed

    Crepaz, Herbert; Ley, Li Yuan; Dumke, Rainer

    2015-01-01

    Atom sensing based on Faraday rotation is an indispensable method for precision measurements, universally suitable for both hot and cold atomic systems. Here we demonstrate an all-optical magnetometer where the optical cell for Faraday rotation spectroscopy is augmented with a low finesse cavity. Unlike in previous experiments, where specifically designed multipass cells had been employed, our scheme allows to use conventional, spherical vapour cells. Spherical shaped cells have the advantage that they can be effectively coated inside with a spin relaxation suppressing layer providing long spin coherence times without addition of a buffer gas. Cavity enhancement shows in an increase in optical polarization rotation and sensitivity compared to single-pass configurations. PMID:26481853

  17. Cavity enhanced atomic magnetometry

    NASA Astrophysics Data System (ADS)

    Crepaz, Herbert; Ley, Li Yuan; Dumke, Rainer

    2015-10-01

    Atom sensing based on Faraday rotation is an indispensable method for precision measurements, universally suitable for both hot and cold atomic systems. Here we demonstrate an all-optical magnetometer where the optical cell for Faraday rotation spectroscopy is augmented with a low finesse cavity. Unlike in previous experiments, where specifically designed multipass cells had been employed, our scheme allows to use conventional, spherical vapour cells. Spherical shaped cells have the advantage that they can be effectively coated inside with a spin relaxation suppressing layer providing long spin coherence times without addition of a buffer gas. Cavity enhancement shows in an increase in optical polarization rotation and sensitivity compared to single-pass configurations.

  18. Spin-polarized dark state free CPT state preparation with co-propagating left and right circularly polarized lasers.

    PubMed

    Zhang, Yi; Qu, Suping; Gu, Sihong

    2012-03-12

    We have developed and experimentally studied a coherent population trapping (CPT) state preparation scheme for atomic clock application with co-propagating left and right circularly polarized lasers. With realization of constructive interference and spin-polarized dark state free in CPT state preparation, we have obtained CPT resonance signal 3 times larger than that of the conventional scheme used in atomic clock. Polarization fluctuations and CPT signal sensitivity to laser power behaviors are both improved with the scheme. Our study reveals that it is a promising candidate for both normal-size and chip-scale CPT atomic clocks. PMID:22418521

  19. Probing absolute spin polarization at the nanoscale.

    PubMed

    Eltschka, Matthias; Jäck, Berthold; Assig, Maximilian; Kondrashov, Oleg V; Skvortsov, Mikhail A; Etzkorn, Markus; Ast, Christian R; Kern, Klaus

    2014-12-10

    Probing absolute values of spin polarization at the nanoscale offers insight into the fundamental mechanisms of spin-dependent transport. Employing the Zeeman splitting in superconducting tips (Meservey-Tedrow-Fulde effect), we introduce a novel spin-polarized scanning tunneling microscopy that combines the probing capability of the absolute values of spin polarization with precise control at the atomic scale. We utilize our novel approach to measure the locally resolved spin polarization of magnetic Co nanoislands on Cu(111). We find that the spin polarization is enhanced by 65% when increasing the width of the tunnel barrier by only 2.3 Å due to the different decay of the electron orbitals into vacuum. PMID:25423049

  20. Acting Atoms.

    ERIC Educational Resources Information Center

    Farin, Susan Archie

    1997-01-01

    Describes a fun game in which students act as electrons, protons, and neutrons. This activity is designed to help students develop a concrete understanding of the abstract concept of atomic structure. (DKM)

  1. Kinetic Atom.

    ERIC Educational Resources Information Center

    Wilson, David B.

    1981-01-01

    Surveys the research of scientists like Joule, Kelvin, Maxwell, Clausius, and Boltzmann as it comments on the basic conceptual issues involved in the development of a more precise kinetic theory and the idea of a kinetic atom. (Author/SK)

  2. Newton's Atom

    NASA Astrophysics Data System (ADS)

    Chaney, Andrea; Espinosa, James; Espinosa, James

    2006-10-01

    At the turn of the twentieth century, physicists and chemists were developing atomic models. Some of the phenomena that they had to explain were the periodic table, the stability of the atom, and the emission spectra. Niels Bohr is known as making the first modern picture that accounted for these. Unknown to much of the physics community is the work of Walter Ritz. His model explained more emission spectra and predates Bohr's work. We will fit several spectra using Ritz's magnetic model for the atom. The problems of stability and chemical periodicity will be shown to be challenges that this model has difficulty solving, but we will present some potentially useful adaptations to the Ritzian atom that can account for them.

  3. Proceedings of the workshop on polarized targets in storage rings

    SciTech Connect

    Holt, R.J.

    1984-08-01

    Polarization phenomena have played an increasingly important part in the study of nuclei and nucleons in recent years. Polarization studies have been hampered by the relatively few and rather fragile polarized targets which are presently available. The concept of polarized gas targets in storage rings opens a much wider range of possibilities than is available in the external target geometry. This novel method will represent a considerable advance in nuclear physics and will continue to receive much attention in plans for future facilities. An internal, polarized-target station is being planned for the cooler ring at the Indiana University Cyclotron Facility. Internal targets are compatible with recent designs of electron accelerators proposed by the Massachusetts Institute of Technology and the Southeastern Universities Research Association. The key to nuclear-science programs based on internal targets pivots on recent developments in polarized atomic beam methods, which include the more recent laser-driven polarized targets. The workshop drew together a unique group of physicists in the fields of high-energy, nuclear and atomic physics. The meeting was organized in a manner that stimulated discussion among the 58 participants and focused on developments in polarized target technology and the underlying atomic physics. An impressive array of future possibilities for polarized targets as well as current developments in polarized target technology were discussed at the workshop. Abstracts of individual items from the workshop were prepared separately for the data base.

  4. Polarity continuation and frustration in ZnSe nanospirals

    PubMed Central

    Li, Luying; Tu, Fanfan; Jin, Lei; Choy, Wallace C. H.; Gao, Yihua; Wang, Jianbo

    2014-01-01

    ZnSe nanospirals including structures with polarity continuation and polarity frustration are simultaneously observed at atomic resolution. Through careful analysis of polarity within each dumbbell based on aberration-corrected high-angle annular-dark-field imaging, polarity continuation across parallel polytype interfaces as well as the surrounding Z-shape faulted dipoles is verified. Moreover, polarity frustration across regions with different stacking sequence, which would lead to accumulations of boundary interface charges in the triangular-shaped mixed regions with potential optoelectronic applications, is carefully studied. PMID:25502957

  5. Light polarization experiments with a diode laser pointer

    NASA Astrophysics Data System (ADS)

    Benenson, Raymond E.

    2000-01-01

    Polarized light has many uses: glare reduction, stress analysis, microscope image enhancement, thin-film characterization, astronomy, saccharimetry, and atomic spectroscopy. Here we discuss introductory polarized light measurements in which a diode laser pointer replaces the more frequently used polarized He-Ne laser. A diode laser has been used in introductory optics experiments, and in a more advanced polarization-reflection experiment. Its strong collimated beam is completely polarized and, being free of infrared radiation, it permits Polaroid sheets to be used successfully with semiconductor detectors.

  6. Cold Atoms

    NASA Astrophysics Data System (ADS)

    Bellac, Michel Le

    2014-11-01

    This chapter and the following one address collective effects of quantum particles, that is, the effects which are observed when we put together a large number of identical particles, for example, electrons, helium-4 or rubidium-85 atoms. We shall see that quantum particles can be classified into two categories, bosons and fermions, whose collective behavior is radically different. Bosons have a tendency to pile up in the same quantum state, while fermions have a tendency to avoid each other. We say that bosons and fermions obey two different quantum statistics, the Bose-Einstein and the Fermi-Dirac statistics, respectively. Temperature is a collective effect, and in Section 5.1 we shall explain the concept of absolute temperature and its relation to the average kinetic energy of molecules. We shall describe in Section 5.2 how we can cool atoms down thanks to the Doppler effect, and explain how cold atoms can be used to improve the accuracy of atomic clocks by a factor of about 100. The effects of quantum statistics are prominent at low temperatures, and atom cooling will be used to obtain Bose-Einstein condensates at low enough temperatures, when the atoms are bosons.

  7. Polar Color

    NASA Technical Reports Server (NTRS)

    2004-01-01

    [figure removed for brevity, see original site]

    Released 3 May 2004 This nighttime visible color image was collected on January 1, 2003 during the Northern Summer season near the North Polar Troughs.

    This daytime visible color image was collected on September 4, 2002 during the Northern Spring season in Vastitas Borealis. The THEMIS VIS camera is capable of capturing color images of the martian surface using its five different color filters. In this mode of operation, the spatial resolution and coverage of the image must be reduced to accommodate the additional data volume produced from the use of multiple filters. To make a color image, three of the five filter images (each in grayscale) are selected. Each is contrast enhanced and then converted to a red, green, or blue intensity image. These three images are then combined to produce a full color, single image. Because the THEMIS color filters don't span the full range of colors seen by the human eye, a color THEMIS image does not represent true color. Also, because each single-filter image is contrast enhanced before inclusion in the three-color image, the apparent color variation of the scene is exaggerated. Nevertheless, the color variation that does appear is representative of some change in color, however subtle, in the actual scene. Note that the long edges of THEMIS color images typically contain color artifacts that do not represent surface variation.

    Image information: VIS instrument. Latitude 79, Longitude 346 East (14 West). 19 meter/pixel resolution.

    Note: this THEMIS visual image has not been radiometrically nor geometrically calibrated for this preliminary release. An empirical correction has been performed to remove instrumental effects. A linear shift has been applied in the cross-track and down-track direction to approximate spacecraft and planetary motion. Fully calibrated and geometrically projected images will be released through the Planetary Data System in accordance with

  8. Penta prism laser polarizer.

    PubMed

    Lotem, H; Rabinovitch, K

    1993-04-20

    A novel type of laser prism polarizer is proposed. The polarizer is characterized by a high transmission efficiency, a high optical damage threshold, and a high extinction ratio. The polarizer is shaped like a regular penta prism and, thus, it is a constant deviation angle device. Polarization effects occur upon the two internal cascade reflections in the prism. Anisotropic and Isotropic types of the polarizer are discussed. The isotropic polarizer is a prism made of a high refractive-index glass coated by multilayer polarization-type dielectric coatings. Efficient s-state polarization is obtained because of p-state leakage upon the two internal cascade reflections. The anisotropic polarizer is made of a birefringent crystal in which angular polarization splitting is obtained by the bireflectance (double-reflection) effect. Fanning of a laser beam into up to eight polarized beams is possible in a prism made of a biaxial crystal. PMID:20820335

  9. Evaporative cooling of potassium atoms

    NASA Astrophysics Data System (ADS)

    Inouye, Shin; Kishimoto, Tetsuo; Kobayashi, Jun; Aikawa, Kiyotaka; Noda, Kai; Arae, Takuto; Ueda, Masahito

    2007-06-01

    Recent advances in manipulating interactions between ultracold atoms opened up various new possibilities. One of the major goal of the field is to produce ultracold polar molecules. By utilizing a magnetic field induced Feshbach resonance, it is possible to produce heteronuclear molecules from a degenerate gas mixture. We are setting up an experiment to produce a degenerate gas mixture of fermionic alkali atoms, lithium-6 and potassium-40. Fermionic atoms are good candidate for minimizing the expected inelastic loss at the Feshbach resonance. For keeping the system as simple as possible, we decided to use bosonic potassium (potassium-41) as a coolant, and sympathetically cool the fermionic species. We will present our experimental setup and initial results for evaporatively cooling bosonic potassium atoms.

  10. Non-coherent continuum scattering as a line polarization mechanism

    SciTech Connect

    Del Pino Alemán, T.; Manso Sainz, R.; Trujillo Bueno, J. E-mail: rsainz@iac.es

    2014-03-20

    Line scattering polarization can be strongly affected by Rayleigh scattering at neutral hydrogen and Thomson scattering at free electrons. Often a depolarization of the continuum results, but the Doppler redistribution produced by the continuum scatterers, which are light (hence, fast), induces more complex interactions between the polarization in spectral lines and in the continuum. Here we formulate and solve the radiative transfer problem of scattering line polarization with non-coherent continuum scattering consistently. The problem is formulated within the spherical tensor representation of atomic and light polarization. The numerical method of solution is a generalization of the Accelerated Lambda Iteration that is applied to both the atomic system and the radiation field. We show that the redistribution of the spectral line radiation due to the non-coherence of the continuum scattering may modify the shape of the emergent fractional linear polarization patterns significantly, even yielding polarization signals above the continuum level in intrinsically unpolarizable lines.

  11. Inducing electric polarization in ultrathin insulating layers

    NASA Astrophysics Data System (ADS)

    Martinez-Castro, Jose; Piantek, Marten; Persson, Mats; Serrate, David; Hirjibehedin, Cyrus F.

    Studies of ultrathin polar oxide films have attracted the interest of researchers for a long time due to their different properties compared to bulk materials. However they present several challenges such as the difficulty in the stabilization of the polar surfaces and the limited success in tailoring their properties. Moreover, recently developed Van der Waals materials have shown that the stacking of 2D-layers trigger new collective states thanks to the interaction between layers. Similarly, interface phenomena emerge in polar oxides, like induced ferroelectricity. This represents a promising way for the creation of new materials with customized properties that differ from those of the isolated layers. Here we present a new approach for the fabrication and study of atomically thin insulating films. We show that the properties of insulating polar layers of sodium chloride (NaCl) can be engineered when they are placed on top of a charge modulated template of copper nitride (Cu2N). STM studies carried out in ultra-high vacuum and at low temperatures over NaCl/Cu2N/Cu(001) show that we are able to build up and stabilize interfaces of polar surface at the limit of one atomic layer showing new properties not present before at the atomic scale.

  12. LINE-INTERLOCKING EFFECTS ON POLARIZATION IN SPECTRAL LINES BY RAYLEIGH AND RAMAN SCATTERING

    SciTech Connect

    Sampoorna, M.; Nagendra, K. N.; Stenflo, J. O. E-mail: knn@iiap.res.in

    2013-06-20

    The polarized spectrum of the Sun and stars is formed from the scattering of anisotropic radiation on atoms. Interpretation of this spectrum requires the solution of polarized line transfer in multilevel atomic systems. While sophisticated quantum theories of polarized line formation in multilevel atomic systems exist, they are limited by the approximation of complete frequency redistribution in scattering. The partial frequency redistribution (PRD) in line scattering is a necessary component in modeling the polarized spectra of strong lines. The polarized PRD line scattering theories developed so far confine themselves to a two-level or a two-term atom model. In this paper, we present a heuristic approach to the problem of polarized line formation in multilevel atoms taking into account the effects of PRD and a weak magnetic field. Starting from the unpolarized PRD multilevel atom approach of Hubeny et al., we incorporate the polarization state of the radiation field. However, the lower level polarization is neglected. Two iterative methods of solving the polarized PRD line transfer in multilevel atoms are also presented. Taking the example of a five-level Ca II atom model, we present illustrative results for an isothermal one-dimensional model atmosphere.

  13. Polarization dependence of double-resonance optical pumping and electromagnetically induced transparency in the 5S{sub 1/2}-5P{sub 3/2}-5D{sub 5/2} transition of {sup 87}Rb atoms

    SciTech Connect

    Moon, Han Seb; Noh, Heung-Ryoul

    2011-09-15

    The polarization dependence of double-resonance optical pumping (DROP) in the ladder-type electromagnetically induced transparency (EIT) of the 5S{sub 1/2}-5P{sub 3/2}-5D{sub 5/2} transition of {sup 87}Rb atoms is studied. The transmittance spectra in the 5S{sub 1/2}(F=2)-5P{sub 3/2}(F'=3)-5D{sub 5/2}(F''=2,3,4) transition were observed as caused by EIT, DROP, and saturation effects in the various polarization combinations between the probe and coupling lasers. The features of the double-structure transmittance spectra in the 5S{sub 1/2}(F=2)-5P{sub 3/2}(F'=3)-5D{sub 5/2}(F''=4) cycling transition were attributed to the difference in saturation effect according to the transition routes between the Zeeman sublevels and the EIT according to the two-photon transition probability.

  14. Polarized Light in Astronomy.

    ERIC Educational Resources Information Center

    King, D. J.

    1983-01-01

    The application of very sensitive electronic detecting devices during the last decade has revolutionized and revitalized the study of polarization in celestial objects. The nature of polarization, how polaroids work, interstellar polarization, dichroic filters, polarization by scattering, and modern polarimetry are among the topics discussed. (JN)

  15. Linearly polarized fiber amplifier

    DOEpatents

    Kliner, Dahv A.; Koplow, Jeffery P.

    2004-11-30

    Optically pumped rare-earth-doped polarizing fibers exhibit significantly higher gain for one linear polarization state than for the orthogonal state. Such a fiber can be used to construct a single-polarization fiber laser, amplifier, or amplified-spontaneous-emission (ASE) source without the need for additional optical components to obtain stable, linearly polarized operation.

  16. Atomic research

    NASA Technical Reports Server (NTRS)

    Hadaway, James B.; Connatser, Robert; Cothren, Bobby; Johnson, R. B.

    1993-01-01

    Work performed by the University of Alabama in Huntsville's (UAH) Center for Applied Optics (CAO) entitled Atomic Research is documented. Atomic oxygen (AO) effects on materials have long been a critical concern in designing spacecraft to withstand exposure to the Low Earth Orbit (LEO) environment. The objective of this research effort was to provide technical expertise in the design of instrumentation and experimental techniques for analyzing materials exposed to atomic oxygen in accelerated testing at NASA/MSFC. Such testing was required to answer fundamental questions concerning Space Station Freedom (SSF) candidate materials and materials exposed to atomic oxygen aboard the Long-Duration Exposure Facility (LDEF). The primary UAH task was to provide technical design, review, and analysis to MSFC in the development of a state-of-the-art 5eV atomic oxygen beam facility required to simulate the RAM-induced low earth orbit (LEO) AO environment. This development was to be accomplished primarily at NASA/MSFC. In support of this task, contamination effects and ultraviolet (UV) simulation testing was also to be carried out using NASA/MSFC facilities. Any materials analysis of LDEF samples was to be accomplished at UAH.

  17. Actuated atomizer

    NASA Technical Reports Server (NTRS)

    Tilton, Charles (Inventor); Weiler, Jeff (Inventor); Palmer, Randall (Inventor); Appel, Philip (Inventor)

    2008-01-01

    An actuated atomizer is adapted for spray cooling or other applications wherein a well-developed, homogeneous and generally conical spray mist is required. The actuated atomizer includes an outer shell formed by an inner ring; an outer ring; an actuator insert and a cap. A nozzle framework is positioned within the actuator insert. A base of the nozzle framework defines swirl inlets, a swirl chamber and a swirl chamber. A nozzle insert defines a center inlet and feed ports. A spool is positioned within the coil housing, and carries the coil windings having a number of turns calculated to result in a magnetic field of sufficient strength to overcome the bias of the spring. A plunger moves in response to the magnetic field of the windings. A stop prevents the pintle from being withdrawn excessively. A pintle, positioned by the plunger, moves between first and second positions. In the first position, the head of the pintle blocks the discharge passage of the nozzle framework, thereby preventing the atomizer from discharging fluid. In the second position, the pintle is withdrawn from the swirl chamber, allowing the atomizer to release atomized fluid. A spring biases the pintle to block the discharge passage. The strength of the spring is overcome, however, by the magnetic field created by the windings positioned on the spool, which withdraws the plunger into the spool and further compresses the spring.

  18. Nondiffracting transversally polarized beam.

    PubMed

    Yuan, G H; Wei, S B; Yuan, X-C

    2011-09-01

    Generation of a nondiffracting transversally polarized beam by means of transmitting an azimuthally polarized beam through a multibelt spiral phase hologram and then highly focusing by a high-NA lens is presented. A relatively long depth of focus (∼4.84λ) of the electric field with only radial and azimuthal components is achieved. The polarization of the wavefront near the focal plane is analyzed in detail by calculating the Stokes polarization parameters. It is found that the polarization is spatially varying and entirely transversally polarized, and the polarization singularity disappears at the beam center, which makes the central bright channel possible. PMID:21886250

  19. Atom Interferometry

    SciTech Connect

    Kasevich, Mark

    2008-05-08

    Atom de Broglie wave interferometry has emerged as a tool capable of addressing a diverse set of questions in gravitational and condensed matter physics, and as an enabling technology for advanced sensors in geodesy and navigation. This talk will review basic principles, then discuss recent applications and future directions. Scientific applications to be discussed include measurement of G (Newton's constant), tests of the Equivalence Principle and post-Newtonian gravity, and study of the Kosterlitz-Thouless phase transition in layered superfluids. Technology applications include development of precision gyroscopes and gravity gradiometers. The talk will conclude with speculative remarks looking to the future: Can atom interference methods be used to detect gravity waves? Can non-classical (entangled/squeezed state) atom sources lead to meaningful sensor performance improvements?

  20. Atom Interferometry

    SciTech Connect

    Mark Kasevich

    2008-05-07

    Atom de Broglie wave interferometry has emerged as a tool capable of addressing a diverse set of questions in gravitational and condensed matter physics, and as an enabling technology for advanced sensors in geodesy and navigation. This talk will review basic principles, then discuss recent applications and future directions. Scientific applications to be discussed include measurement of G (Newton’s constant), tests of the Equivalence Principle and post-Newtonian gravity, and study of the Kosterlitz-Thouless phase transition in layered superfluids. Technology applications include development of precision gryoscopes and gravity gradiometers. The talk will conclude with speculative remarks looking to the future: Can atom interference methods be sued to detect gravity waves? Can non-classical (entangled/squeezed state) atom sources lead to meaningful sensor performance improvements?

  1. Atom Interferometry

    ScienceCinema

    Mark Kasevich

    2010-01-08

    Atom de Broglie wave interferometry has emerged as a tool capable of addressing a diverse set of questions in gravitational and condensed matter physics, and as an enabling technology for advanced sensors in geodesy and navigation. This talk will review basic principles, then discuss recent applications and future directions. Scientific applications to be discussed include measurement of G (Newton?s constant), tests of the Equivalence Principle and post-Newtonian gravity, and study of the Kosterlitz-Thouless phase transition in layered superfluids. Technology applications include development of precision gryoscopes and gravity gradiometers. The talk will conclude with speculative remarks looking to the future: Can atom interference methods be sued to detect gravity waves? Can non-classical (entangled/squeezed state) atom sources lead to meaningful sensor performance improvements?

  2. Quantum teleportation with atoms trapped in cavities

    SciTech Connect

    Cho, Jaeyoon; Lee, Hai-Woong

    2004-09-01

    We propose a scheme to implement the quantum teleportation protocol with single atoms trapped in cavities. The scheme is based on the adiabatic passage and the polarization measurement. We show that it is possible to teleport the internal state of an atom trapped in a cavity to an atom trapped in another cavity with the success probability of 1/2 and the fidelity of 1. The scheme is resistant to a number of considerable imperfections such as the violation of the Lamb-Dicke condition, weak atom-cavity coupling, spontaneous emission, and detection inefficiency.

  3. Crossed elliptical polarization undulator

    SciTech Connect

    Sasaki, Shigemi

    1997-05-01

    The first switching of polarization direction is possible by installing two identical helical undulators in series in a same straight section in a storage ring. By setting each undulator in a circular polarization mode in opposite handedness, one can obtain linearly polarized radiation with any required polarization direction depending on the modulator setting between two undulators. This scheme can be used without any major degradation of polarization degree in any low energy low emittance storage ring.

  4. Polarization-balanced beamsplitter

    DOEpatents

    Decker, D.E.

    1998-02-17

    A beamsplitter assembly is disclosed that includes several beamsplitter cubes arranged to define a plurality of polarization-balanced light paths. Each polarization-balanced light path contains one or more balanced pairs of light paths, where each balanced pair of light paths includes either two transmission light paths with orthogonal polarization effects or two reflection light paths with orthogonal polarization effects. The orthogonal pairing of said transmission and reflection light paths cancels polarization effects otherwise caused by beamsplitting. 10 figs.

  5. Polarization-balanced beamsplitter

    DOEpatents

    Decker, Derek E.

    1998-01-01

    A beamsplitter assembly that includes several beamsplitter cubes arranged to define a plurality of polarization-balanced light paths. Each polarization-balanced light path contains one or more balanced pairs of light paths, where each balanced pair of light paths includes either two transmission light paths with orthogonal polarization effects or two reflection light paths with orthogonal polarization effects. The orthogonal pairing of said transmission and reflection light paths cancels polarization effects otherwise caused by beamsplitting.

  6. The impacts of surface polarity on the solubility of nanoparticle.

    PubMed

    Zhu, Jianzhuo; Ou, Xinwen; Su, Jiguo; Li, Jingyuan

    2016-07-28

    In order to study the dependence of water solubility and hydration behavior of nanoparticles on their surface polarity, we designed polar nanoparticles with varying surface polarity by assigning atomic partial charge to the surface of C60. The water solubility of the nanoparticle is enhanced by several orders of magnitude after the introduction of surface polarity. Nevertheless, when the atomic partial charge grows beyond a certain value (qM), the solubility continuously decreases to the level of nonpolar nanoparticle. It should be noted that such qM is comparable with atomic partial charge of a variety of functional groups. The hydration behaviors of nanoparticles were then studied to investigate the non-monotonic dependence of solubility on the surface polarity. The interaction between the polar nanoparticle and the hydration water is stronger than the nonpolar counterpart, which should facilitate the dissolution of the nanoparticles. On the other hand, the surface polarity also reduces the interaction of hydration water with the other water molecules and enhances the interaction between the nanoparticles which may hinder their dispersion. Besides, the introduction of surface polarity disturbs and even rearranges the hydration structure of nonpolar nanoparticle. Interestingly, the polar nanoparticle with less ordered hydration structure tends to have higher water solubility. PMID:27475378

  7. The impacts of surface polarity on the solubility of nanoparticle

    NASA Astrophysics Data System (ADS)

    Zhu, Jianzhuo; Ou, Xinwen; Su, Jiguo; Li, Jingyuan

    2016-07-01

    In order to study the dependence of water solubility and hydration behavior of nanoparticles on their surface polarity, we designed polar nanoparticles with varying surface polarity by assigning atomic partial charge to the surface of C60. The water solubility of the nanoparticle is enhanced by several orders of magnitude after the introduction of surface polarity. Nevertheless, when the atomic partial charge grows beyond a certain value (qM), the solubility continuously decreases to the level of nonpolar nanoparticle. It should be noted that such qM is comparable with atomic partial charge of a variety of functional groups. The hydration behaviors of nanoparticles were then studied to investigate the non-monotonic dependence of solubility on the surface polarity. The interaction between the polar nanoparticle and the hydration water is stronger than the nonpolar counterpart, which should facilitate the dissolution of the nanoparticles. On the other hand, the surface polarity also reduces the interaction of hydration water with the other water molecules and enhances the interaction between the nanoparticles which may hinder their dispersion. Besides, the introduction of surface polarity disturbs and even rearranges the hydration structure of nonpolar nanoparticle. Interestingly, the polar nanoparticle with less ordered hydration structure tends to have higher water solubility.

  8. Neutron polarizers based on polarized ^3He

    NASA Astrophysics Data System (ADS)

    Gentile, T. R.; Jones, G. L.; Thompson, A. K.; Fei, X.; Keith, C. D.; Rich, D.; Snow, W. M.; Penttila, S.

    1997-10-01

    Research is underway at NIST, Indiana Univ., and LANL to develop neutron polarizers and analyzers based on polarized ^3He. Such devices, which rely on the strong spin dependence of the neutron capture cross section by polarized ^3He, have applications in weak interaction physics and materials science. In addition, the technology for polarized ^3He production is directly applicable to polarized gas MRI of lungs, and polarized targets. Our program, which includes both the spin-exchange and metastability-exchange optical pumping methods, will be reviewed. Spin-exchange has been used to analyze a polarized cold neutron beam at NIST, and also for lung imaging in collaboration with the Univ. of Pennsylvania. In the metastable method, the ^3He is polarized at low pressure, and must be substantially compressed. A piston compressor has been designed for this goal at Indiana Univ. and is under construction. At NIST we have compressed polarized gas using an apparatus that is based on a modified commercial diaphragm pump.

  9. Polarized EMC Effect in Nuclei

    SciTech Connect

    Ian Cloet; A. W. Thomas; W. Bentz

    2006-06-05

    The discovery of the EMC effect and the proton spin crisis by the European Muon Collaboration are two of the standout experiments of the last 25 years. It is therefore surprising that there has been no experimental and little theoretical investigation of the spin structure functions of atomic nuclei. To address this we present results for the spin-dependent structure functions of nuclei. The quark degrees of freedom in nuclei are accessed via the convolution formalism. Where the nucleon bound state is obtained by solving the relativistic Faddeev equation, and a relativistic shell model is used to model the atomic nucleus. We find the important result that the medium modifications to the polarized structure functions are about twice that of the unpolarized case.

  10. Beam transport of low temperature atomic hydrogen

    NASA Astrophysics Data System (ADS)

    Kaufman, W. A.

    1993-12-01

    Analytic calculations and particle tracking simulations are presented for a polarized atomic hydrogen beam produced by extraction from an ultra-cold (T=300 mK) helium film coated cell in a large solenoidal magnetic field (12 T). Initial focusing of states 1 and 2 by the solenoidal field and subsequent focusing by a sextupole are examined within the constraints imposed by the requirements of the polarized jet for the experiments NEPTUN and NEPTUN-A at UNK.

  11. Magnetic measurements with atomic-plane resolution.

    PubMed

    Rusz, Ján; Muto, Shunsuke; Spiegelberg, Jakob; Adam, Roman; Tatsumi, Kazuyoshi; Bürgler, Daniel E; Oppeneer, Peter M; Schneider, Claus M

    2016-01-01

    Rapid development of magnetic nanotechnologies calls for experimental techniques capable of providing magnetic information with subnanometre spatial resolution. Available probes of magnetism either detect only surface properties, such as spin-polarized scanning tunnelling microscopy, magnetic force microscopy or spin-polarized low-energy electron microscopy, or they are bulk probes with limited spatial resolution or quantitativeness, such as X-ray magnetic circular dichroism or classical electron magnetic circular dichroism (EMCD). Atomic resolution EMCD methods have been proposed, although not yet experimentally realized. Here, we demonstrate an EMCD technique with an atomic size electron probe utilizing a probe-corrected scanning transmission electron microscope in its standard operation mode. The crucial element of the method is a ramp in the phase of the electron beam wavefunction, introduced by a controlled beam displacement. We detect EMCD signals with atomic-plane resolution, thereby bringing near-atomic resolution magnetic circular dichroism spectroscopy to hundreds of laboratories worldwide. PMID:27578421

  12. The physics of spin polarized gases

    NASA Astrophysics Data System (ADS)

    Cates, Gordon D.

    1995-01-01

    Most of our research was connected either directly or indirectly to the study of spin polarized atoms and nuclei, and their applications. In most cases we used lasers to optically pump, and hence polarize, alkali-metal vapors. Spin-exchange collisions were used to transfer the angular momentum to other systems. Of particular interest was our continuing study of the polarization of noble gas nuclei, which are characterized by extremely long spin relaxation times of minutes to many days. During this past research period we have demonstrated several applications of polarized noble gas nuclei that may have important implications for such diverse areas as nondestructive testing and medical diagnostics, as well as many areas in fundamental research. Of particular note is the use of spin-exchange polarized He-3 and Xe-129 for magnetic resonance imaging. At present, our imaging work has focused on the lungs of small animals such as mice and guinea pigs. We believe, however, that our technique would also be useful for nondestructive testing. We have also continued our study of Xe that is polarized in the gaseous state, and subsequently frozen. This novel technique for producing a highly polarized solid has received considerable attention in the NMR community.

  13. Studies of Interstellar and Circumstellar Magnetic Field with Aligned Atoms

    NASA Astrophysics Data System (ADS)

    Lazarian, A.; Yan, H.

    2004-12-01

    Population of levels of the hyperfine and fine split ground state of an atom is affected by radiative transitions induced by anisotropic radiation flux. Such aligned atoms precess in the external magnetic field and this affects properties of polarized radiation arising from both scattering and absorption by atoms. As the result the degree of light polarization depends on the direction of the magnetic field. This provides a new tool for studies of astrophysical magnetic fields using optical and UV polarimetry. We provide calculations for several atoms and ions that can be used to study magnetic fields in interplanetary medium, interstellar medius, circumstellar regions and quasars.

  14. Constructive polarization modulation for coherent population trapping clock

    SciTech Connect

    Yun, Peter Danet, Jean-Marie; Holleville, David; Clercq, Emeric de; Guérandel, Stéphane

    2014-12-08

    We propose a constructive polarization modulation scheme for atomic clocks based on coherent population trapping (CPT). In this scheme, the polarization of a bichromatic laser beam is modulated between two opposite circular polarizations to avoid trapping the atomic populations in the extreme Zeeman sublevels. We show that if an appropriate phase modulation between the two optical components of the bichromatic laser is applied synchronously, the two CPT dark states which are produced successively by the alternate polarizations add constructively. Measured CPT resonance contrasts up to 20% in one-pulse CPT and 12% in two-pulse Ramsey-CPT experiments are reported, demonstrating the potential of this scheme for applications to high performance atomic clocks.

  15. Nuclear spin polarized H and D by means of spin-exchange optical pumping

    NASA Astrophysics Data System (ADS)

    Stenger, Jörn; Grosshauser, Carsten; Kilian, Wolfgang; Nagengast, Wolfgang; Ranzenberger, Bernd; Rith, Klaus; Schmidt, Frank

    1998-01-01

    Optically pumped spin-exchange sources for polarized hydrogen and deuterium atoms have been demonstrated to yield high atomic flow and high electron spin polarization. For maximum nuclear polarization the source has to be operated in spin temperature equilibrium, which has already been demonstrated for hydrogen. In spin temperature equilibrium the nuclear spin polarization PI equals the electron spin polarization PS for hydrogen and is even larger than PS for deuterium. We discuss the general properties of spin temperature equilibrium for a sample of deuterium atoms. One result are the equations PI=4PS/(3+PS2) and Pzz=PSṡPI, where Pzz is the nuclear tensor polarization. Furthermore we demonstrate that the deuterium atoms from our source are in spin temperature equilibrium within the experimental accuracy.

  16. Atomic rivals

    SciTech Connect

    Goldschmidt, B.

    1990-01-01

    This book is a memoir of rivalries among the Allies over the bomb, by a participant and observer. Nuclear proliferation began in the uneasy wartime collaboration of the United States, England, Canada, and Free France to produce the atom bomb. Through the changes of history, a young French chemist had a role in almost every act of this international drama. This memoir is based on Goldschmidt's own recollections, interviews with other leading figures, and 3,000 pages of newly declassified documents in Allied archives. From his own start as Marie Curie's lab assistant, Goldschmidt's career was closely intertwined with Frances complicated rise to membership in the nuclear club. As a refugee from the Nazis, he became part of the wartime nuclear energy project in Canada and found himself the only French scientist to work (although briefly) on the American atom bomb project.

  17. Atomic arias

    NASA Astrophysics Data System (ADS)

    Crease, Robert P.

    2009-01-01

    The American composer John Adams uses opera to dramatize controversial current events. His 1987 work Nixon in China was about the landmark meeting in 1972 between US President Richard Nixon and Chairman Mao Zedong of China; The Death of Klinghoffer (1991) was a musical re-enactment of an incident in 1985 when Palestinian terrorists kidnapped and murdered a wheelchair-bound Jewish tourist on a cruise ship. Adams's latest opera, Doctor Atomic, is also tied to a controversial event: the first atomic-bomb test in Alamogordo, New Mexico, on 16 June 1945. The opera premièred in San Francisco in 2005, had a highly publicized debut at the Metropolitan Opera in New York in 2008, and will have another debut on 25 February - with essentially the same cast - at the English National Opera in London.

  18. Development of an optically pumped polarized deuterium target

    SciTech Connect

    Young, L.; Holt, R.J.; Green, M.C.; Kowalczyk, R.

    1987-01-01

    The development of a polarized deuterium target for internal use at an electron storage ring is of great interest for fundamental studies in nuclear physics. In order to achieve the maximum allowable target thickness, 10/sup 14/ nuclei/cm/sup 2/, consistent with various constraints imposed by the storage ring environment, a flux of 4 x 10/sup 17/ polarized atom/s must be provided. This flux exceeds the capability of conventional atomic beam sources by an order of magnitude. We have been developing an alternative source based upon the spin-exchange optical pumping method in which the flux is limited only by laser power. 7 refs., 1 fig.

  19. Atomic physics

    SciTech Connect

    Livingston, A.E.; Kukla, K.; Cheng, S.

    1995-08-01

    In a collaboration with the Atomic Physics group at Argonne and the University of Toledo, the Atomic Physics group at the University of Notre Dame is measuring the fine structure transition energies in highly-charged lithium-like and helium-like ions using beam-foil spectroscopy. Precise measurements of 2s-2p transition energies in simple (few-electron) atomic systems provide stringent tests of several classes of current atomic- structure calculations. Analyses of measurements in helium-like Ar{sup 16+} have been completed, and the results submitted for publication. A current goal is to measure the 1s2s{sup 3}S{sub 1} - 1s2p{sup 3}P{sub 0} transition wavelength in helium-like Ni{sup 26+}. Measurements of the 1s2s{sup 2}S{sub 1/2} - 1s2p{sup 2}P{sub 1/2,3/2} transition wavelengths in lithium-like Kr{sup 33+} is planned. Wavelength and lifetime measurements in copper-like U{sup 63+} are also expected to be initiated. The group is also participating in measurements of forbidden transitions in helium-like ions. A measurement of the lifetime of the 1s2s{sup 3}S{sub 1} state in Kr{sup 34+} was published recently. In a collaboration including P. Mokler of GSI, Darmstadt, measurements have been made of the spectral distribution of the 2E1 decay continuum in helium-like Kr{sup 34+}. Initial results have been reported and further measurements are planned.

  20. Atomic Magnetometry for fetal Magnetocardiography

    NASA Astrophysics Data System (ADS)

    Sulai, Ibrahim; Walker, Thad; Wakai, Ronald

    2013-05-01

    We present results of using an array of atomic magnetometers in detecting fetal Magnetocardiograms(fMCG). The array consists of four 87-Rb atomic magnetometers operating in the spin exchange relaxation free (SERF) regime. They have a demonstrated sensitivity of 5 - 10 fT /√{ Hz } -limited by the Johnson noise of the magnetic shielding. We report measurements of fMCG on gestational ages as small as 21 weeks and describe the technical challenges and design features that make the measurements possible. We present a method for minimizing the impact of AC Stark Shifts on the magnetometer array performance by relying on diffusion to transport polarized atoms from a pumping region to an AC Stark shift free active region. This work was supported by the NIH.

  1. Scattering of electrons from neon atoms

    NASA Technical Reports Server (NTRS)

    Dasgupta, A.; Bhatia, A. K.

    1984-01-01

    Scattering of electrons from neon atoms is investigated by the polarized-orbital method. The perturbed orbitals calculated with use of the Sternheimer approximation lead to the polarizability 2.803 a(0)-cube in fairly good agreement with the experimental value 2.66 a(0)-cube. Phase shifts for various partial waves are calculated in the exchange, exchange-adiabatic, and polarized-orbital approximations. They are compared with the previous results. The calculated elastic differential, total, and momentum-transfer cross sections are compared with the experimental results. The polarized-orbital approximation yields results which show general improvement over the exchange-adiabatic approximation.

  2. Polarized Light Corridor Demonstrations.

    ERIC Educational Resources Information Center

    Davies, G. R.

    1990-01-01

    Eleven demonstrations of light polarization are presented. Each includes a brief description of the apparatus and the effect demonstrated. Illustrated are strain patterns, reflection, scattering, the Faraday Effect, interference, double refraction, the polarizing microscope, and optical activity. (CW)

  3. Polarization at SLAC

    SciTech Connect

    Woods, M.

    1995-01-01

    A highly polarized electron beam is a key feature. for the Current physics program at SLAC. An electron beam polarization of 80% can now be routinely achieved for typically 5000 hours of machine operation per year. Two main Physics programs utilize the polarized beam. Fixed target experiments in End Station A study the collision of polarized electrons with polarized nuclear targets to elucidate the spin structure of the nucleon and to provide an important test of QCD. Using the SLAC Linear Collider, collisions of polarized electrons with unpolarized positrons allow precise measurements of parity violation in the Z-fermion couplings and provide a very precise measurement of tile weak mixing angle. This paper discusses polarized beam operation at SLAC, and gives an overview of the polarized physics program.

  4. A Translational Polarization Rotator

    NASA Technical Reports Server (NTRS)

    Chuss, David T.; Wollack, Edward J.; Pisano, Giampaolo; Ackiss, Sheridan; U-Yen, Kongpop; Ng, Ming wah

    2012-01-01

    We explore a free-space polarization modulator in which a variable phase introduction between right- and left-handed circular polarization components is used to rotate the linear polarization of the outgoing beam relative to that of the incoming beam. In this device, the polarization states are separated by a circular polarizer that consists of a quarter-wave plate in combination with a wire grid. A movable mirror is positioned behind and parallel to the circular polarizer. As the polarizer-mirror distance is separated, an incident liear polarization will be rotated through an angle that is proportional to the introduced phase delay. We demonstrate a prototype device that modulates Stokes Q and U over a 20% bandwidth.

  5. Anomalously robust valley polarization and valley coherence in bilayer WS2

    PubMed Central

    Zhu, Bairen; Zeng, Hualing; Dai, Junfeng; Gong, Zhirui; Cui, Xiaodong

    2014-01-01

    We report the observation of anomalously robust valley polarization and valley coherence in bilayer WS2. The polarization of the photoluminescence from bilayer WS2 follows that of the excitation source with both circular and linear polarization, and remains even at room temperature. The near-unity circular polarization of the luminescence reveals the coupling of spin, layer, and valley degree of freedom in bilayer system, and the linearly polarized photoluminescence manifests quantum coherence between the two inequivalent band extrema in momentum space, namely, the valley quantum coherence in atomically thin bilayer WS2. This observation provides insight into quantum manipulation in atomically thin semiconductors. PMID:25071178

  6. Quantum magnetism of alkali Rydberg atoms

    NASA Astrophysics Data System (ADS)

    Malinovskaya, Svetlana; Liu, Gengyuan

    2016-05-01

    We discuss a method to control dynamics in many-body spin states of 87Rb Rydberg atoms. The method permits excitation of cold gases and form ordered structures of alkali atoms. It makes use of a two-photon excitation scheme with circularly polarized and linearly chirped pulses. The method aims for controlled quantum state preparation in large ensembles. It is actual for experiments studding the spin hopping dynamics and realization of quantum random walks.

  7. Atomic-level imaging, processing and characterization of semiconductor surfaces

    DOEpatents

    Kazmerski, L.L.

    1995-08-22

    A method for selecting and removing single specific atoms from a solid material surface uses photon biasing to break down bonds that hold the selected atom in the lattice and to reduce barrier effects that hold the atom from transferring to a probe. The photon bias is preferably light or other electromagnetic radiation with a wavelength and frequency that approximately matches the wave function of the target atom species to be removed to induce high energy, selective thermionic-like vibration. An electric field potential is then applied between the probe and the surface of the solid material to pull the atom out of the lattice and to transfer the atom to the probe. Different extrinsic atoms can be installed in the lattice sites that are vacated by the removed atoms by using a photon bias that resonates the extrinsic atom species, reversing polarity of the electric field, and blowing gas comprising the extrinsic atoms through a hollow catheter probe. 8 figs.

  8. Atomic-level imaging, processing and characterization of semiconductor surfaces

    DOEpatents

    Kazmerski, Lawrence L.

    1995-01-01

    A method for selecting and removing single specific atoms from a solid material surface uses photon biasing to break down bonds that hold the selected atom in the lattice and to reduce barrier effects that hold the atom from transferring to a probe. The photon bias is preferably light or other electromagnetic radiation with a wavelength and frequency that approximately matches the wave function of the target atom species to be removed to induce high energy, selective thermionic-like vibration. An electric field potential is then applied between the probe and the surface of the solid material to pull the atom out of the lattice and to transfer the atom to the probe. Different extrinsic atoms can be installed in the lattice sites that are vacated by the removed atoms by using a photon bias that resonates the extrinsic atom species, reversing polarity of the electric field, and blowing gas comprising the extrinsic atoms through a hollow catheter probe.

  9. Polar Ozone Workshop. Abstracts

    NASA Technical Reports Server (NTRS)

    Aikin, Arthur C.

    1988-01-01

    Results of the proceedings of the Polar Ozone Workshop held in Snowmass, CO, on May 9 to 13, 1988 are given. Topics covered include ozone depletion, ozonometry, polar meteorology, polar stratospheric clouds, remote sensing of trace gases, atmospheric chemistry and dynamical simulations.

  10. Hybrid polarization control

    NASA Astrophysics Data System (ADS)

    Gray, George R.; Ibragimov, Edem; Sluz, Joseph; Sova, Raymond

    2005-05-01

    We demonstrate a novel method of polarization control that combines rotatable waveplates (angle control) and variable retarders (retardance control). Such a "hybrid" polarization controller performs far better than conventional controllers, allowing nearly perfect arbitrary-to-arbitrary polarization transformations. We show theoretically that the two control parameters augment one another because they tend to result in orthogonal movements on the Poincaré sphere.

  11. Graphing Polar Curves

    ERIC Educational Resources Information Center

    Lawes, Jonathan F.

    2013-01-01

    Graphing polar curves typically involves a combination of three traditional techniques, all of which can be time-consuming and tedious. However, an alternative method--graphing the polar function on a rectangular plane--simplifies graphing, increases student understanding of the polar coordinate system, and reinforces graphing techniques learned…

  12. Playing with Polarizers.

    ERIC Educational Resources Information Center

    Hecht, Jeff

    1991-01-01

    Discussed is how polarized sunglasses block glare, help spot subtle differences in surfaces, and give a clearer view under water. Information on unpolarized and polarized light is provided. The reasons causing glare to occur and how polarizers decrease glare are discussed. (KR)

  13. Polarity at Many Levels

    ERIC Educational Resources Information Center

    Flannery, Maura C.

    2004-01-01

    An attempt is made to find how polarity arises and is maintained, which is a central issue in development. It is a fundamental attribute of living things and cellular polarity is also important in the development of multicellular organisms and controversial new work indicates that polarization in mammals may occur much earlier than previously…

  14. Bumblebees Learn Polarization Patterns

    PubMed Central

    Foster, James J.; Sharkey, Camilla R.; Gaworska, Alicia V.A.; Roberts, Nicholas W.; Whitney, Heather M.; Partridge, Julian C.

    2014-01-01

    Summary Foraging insect pollinators such as bees must find and identify flowers in a complex visual environment. Bees use skylight polarization patterns for navigation [1–3], a capacity mediated by the polarization-sensitive dorsal rim area (DRA) of their eye [4, 5]. While other insects use polarization sensitivity to identify appropriate habitats [6], oviposition sites, and food sources [7], to date no nonnavigational functions of polarization vision have been identified in bees. Here we investigated the ability of bumblebees (Bombus terrestris) to learn polarization patterns on artificial “flowers” in order to obtain a food reward. We show that foraging bumblebees can learn to discriminate between two differently polarized targets, but only when the target artificial “flower” is viewed from below. A context for these results is provided by polarization imaging of bee-pollinated flowers, revealing the potential for polarization patterns in real flowers. Bees may therefore have the ability to use polarization vision, possibly mediated by their polarization-sensitive DRA, both for navigation and to learn polarization patterns on flowers, the latter being the first nonnavigational function for bee polarization vision to be identified. PMID:24909321

  15. Polarization feedback laser stabilization

    DOEpatents

    Esherick, Peter; Owyoung, Adelbert

    1988-01-01

    A system for locking two Nd:YAG laser oscillators includes an optical path for feeding the output of one laser into the other with different polarizations. Elliptical polarization is incorporated into the optical path so that the change in polarization that occurs when the frequencies coincide may be detected to provide a feedback signal to control one laser relative to the other.

  16. Calculation of polarization effects

    SciTech Connect

    Chao, A.W.

    1983-09-01

    Basically there are two areas of accelerator applications that involve beam polarization. One is the acceleration of a polarized beam (most likely a proton beam) in a synchrotron. Another concerns polarized beams in an electron storage ring. In both areas, numerical techniques have been very useful.

  17. Trap-control system for polarized-electron source

    SciTech Connect

    Agranovich, V.L.; Beloglazov, V.I.; Efimov, V.P.; Kuz'menko, V.S.

    1985-11-01

    An electronic logic system for controlling accumulation and holding of electrons with energies less than 10 eV for polarization is described. A source of polarized electrons based on spin exchange with atoms of polarized hydrogen has been created for physics research on the linear accelerator of the Kharkov Applied Physics Institute. It was necessary to create functional supply and control circuits that feed to the trap electrodes pulsed voltages of given amplitude, polarity and duration. A diagram of the trap-control system is shown.

  18. Heralded entanglement of two remote atoms

    NASA Astrophysics Data System (ADS)

    Krug, Michael; Hofmann, Julian; Ortegel, Norbert; Gerard, Lea; Redeker, Kai; Henkel, Florian; Rosenfeld, Wenjamin; Weber, Markus; Weinfurter, Harald

    2012-06-01

    Entanglement between atomic quantum memories at remote locations will be a key resource for future applications in quantum communication. One possibility to generate such entanglement over large distances is entanglement swapping starting from two quantum memories each entangled with a photon. The photons can be transported to a Bell-state measurement where after the atomic quantum memories are projected onto an entangled state. We have set up two independently operated single atom experiments separated by 20 m. Via a spontaneous decay process each quantum memory, in our case a single Rb-87 atom, emits a single photon whose polarization is entangled with the atomic spin. The photons one emitted from each atom are collected into single-mode optical fibers guided to a non-polarizing 50-50 beam-splitter and detected by avalanche photodetectors. Bunching of indistinguishable photons allows to perform a Bell-state measurement on the photons. Conditioned on the registration of particular two-photon coincidences the spin states of both atoms are measured. The observed correlations clearly prove the entanglement of the two atoms. This is a first step towards creating a basic node of a quantum network as well as a key prerequisite for a future loophole-free test of Bell's inequality.

  19. Detection of J-coupling using atomic magnetometer

    DOEpatents

    Ledbetter, Micah P.; Crawford, Charles W.; Wemmer, David E.; Pines, Alexander; Knappe, Svenja; Kitching, John; Budker, Dmitry

    2015-09-22

    An embodiment of a method of detecting a J-coupling includes providing a polarized analyte adjacent to a vapor cell of an atomic magnetometer; and measuring one or more J-coupling parameters using the atomic magnetometer. According to an embodiment, measuring the one or more J-coupling parameters includes detecting a magnetic field created by the polarized analyte as the magnetic field evolves under a J-coupling interaction.

  20. Diffusive suppression of AC-Stark shifts in atomic magnetometers

    PubMed Central

    Sulai, I. A.; Wyllie, R.; Kauer, M.; Smetana, G. S.; Wakai, R. T.; Walker, T. G.

    2016-01-01

    In atomic magnetometers, the vector AC-Stark shift associated with circularly polarized light generates spatially varying effective magnetic fields, which limit the magnetometer response and serve as sources of noise. We describe a scheme whereby optically pumping a small subvolume of the magnetometer cell and relying on diffusion to transport polarized atoms allows a magnetometer to be operated with minimal sensitivity to the AC-Stark field. © 2013 Optical Society of America PMID:23503278

  1. Atomic-scale control of graphene magnetism by using hydrogen atoms

    NASA Astrophysics Data System (ADS)

    González-Herrero, Héctor; Gómez-Rodríguez, José M.; Mallet, Pierre; Moaied, Mohamed; Palacios, Juan José; Salgado, Carlos; Ugeda, Miguel M.; Veuillen, Jean-Yves; Yndurain, Félix; Brihuega, Iván

    2016-04-01

    Isolated hydrogen atoms absorbed on graphene are predicted to induce magnetic moments. Here we demonstrate that the adsorption of a single hydrogen atom on graphene induces a magnetic moment characterized by a ~20–millielectron volt spin-split state at the Fermi energy. Our scanning tunneling microscopy (STM) experiments, complemented by first-principles calculations, show that such a spin-polarized state is essentially localized on the carbon sublattice opposite to the one where the hydrogen atom is chemisorbed. This atomically modulated spin texture, which extends several nanometers away from the hydrogen atom, drives the direct coupling between the magnetic moments at unusually long distances. By using the STM tip to manipulate hydrogen atoms with atomic precision, it is possible to tailor the magnetism of selected graphene regions.

  2. Atomic-scale control of graphene magnetism by using hydrogen atoms.

    PubMed

    González-Herrero, Héctor; Gómez-Rodríguez, José M; Mallet, Pierre; Moaied, Mohamed; Palacios, Juan José; Salgado, Carlos; Ugeda, Miguel M; Veuillen, Jean-Yves; Yndurain, Félix; Brihuega, Iván

    2016-04-22

    Isolated hydrogen atoms absorbed on graphene are predicted to induce magnetic moments. Here we demonstrate that the adsorption of a single hydrogen atom on graphene induces a magnetic moment characterized by a ~20-millielectron volt spin-split state at the Fermi energy. Our scanning tunneling microscopy (STM) experiments, complemented by first-principles calculations, show that such a spin-polarized state is essentially localized on the carbon sublattice opposite to the one where the hydrogen atom is chemisorbed. This atomically modulated spin texture, which extends several nanometers away from the hydrogen atom, drives the direct coupling between the magnetic moments at unusually long distances. By using the STM tip to manipulate hydrogen atoms with atomic precision, it is possible to tailor the magnetism of selected graphene regions. PMID:27102478

  3. Atomic Clocks

    NASA Astrophysics Data System (ADS)

    Wynands, Robert

    Time is a strange thing. On the one hand it is arguably the most inaccessible physical phenomenon of all: both in that it is impossible to manipulate or modify—for all we know—and in that even after thousands of years mankind's philosophers still have not found a fully satisfying way to understand it. On the other hand, no other quantity can be measured with greater precision. Today's atomic clocks allow us to reproduce the length of the second as the SI unit of time with an uncertainty of a few parts in 1016—orders of magnitude better than any other quantity. In a sense, one can say [1

  4. Velocity distributions of hydrogen atoms and hydroxyl radicals produced through solar photodissociation of water

    NASA Technical Reports Server (NTRS)

    Wu, C. Y. R.; Chen, F. Z.

    1993-01-01

    The velocity distributions of H and OH fragments produced through solar photodissociation of gaseous H2O molecules under collisionless conditions are presented. The calculations are carried out using: the most recently available absolute partial cross sections for the production of H and OH through photodissociation of H2O from its absorption onset at 1860 A down to 500 A; the newly available vibrational and rotational energy distributions of both the excited and ground state OH photofragments; the calculated cross sections for the total dissociation processes; and the integrated solar flux in 10 A increments from 500 to 1860 A in the continuum regions and the specific wavelength and flux at the bright solar lines. The calculated results show that the H atoms and the OH radicals produced exhibit multiple velocity groups. Since most current cometary modeling uses a single velocity of 20 km/sec associated with the photodissociation of H2O, the present results may be useful in interpreting the many peaks observed in the velocity distributions of the H Lyman alpha and H alpha of comets.

  5. Velocity distributions of hydrogen atoms and hydroxyl radicals produced through solar photodissociation of water

    NASA Astrophysics Data System (ADS)

    Wu, C. Y. R.; Chen, F. Z.

    1993-04-01

    The velocity distributions of H and OH fragments produced through solar photodissociation of gaseous H2O molecules under collisionless conditions are presented. The calculations are carried out using: the most recently available absolute partial cross sections for the production of H and OH through photodissociation of H2O from its absorption onset at 1860 A down to 500 A; the newly available vibrational and rotational energy distributions of both the excited and ground state OH photofragments; the calculated cross sections for the total dissociation processes; and the integrated solar flux in 10 A increments from 500 to 1860 A in the continuum regions and the specific wavelength and flux at the bright solar lines. The calculated results show that the H atoms and the OH radicals produced exhibit multiple velocity groups. Since most current cometary modeling uses a single velocity of 20 km/sec associated with the photodissociation of H2O, the present results may be useful in interpreting the many peaks observed in the velocity distributions of the H Lyman alpha and H alpha of comets.

  6. Composition law for polarizers

    NASA Astrophysics Data System (ADS)

    Lages, J.; Giust, R.; Vigoureux, J.-M.

    2008-09-01

    The polarization process when polarizers act on an optical field is studied. We give examples for two kinds of polarizers. The first kind presents an anisotropic absorption—as in a Polaroid film—and the second one is based on total reflection at the interface with a birefringent medium. Using the Stokes vector representation, we determine explicitly the trajectories of the wave light polarization during the polarization process. We find that such trajectories are not always geodesics of the Poincaré sphere as is usually thought. Using the analogy between light polarization and special relativity, we find that the action of successive polarizers on the light wave polarization is equivalent to the action of a single resulting polarizer followed by a rotation achieved, for example, by a device with optical activity. We find a composition law for polarizers similar to the composition law for noncollinear velocities in special relativity. We define an angle equivalent to the relativistic Wigner angle which can be used to quantify the quality of two composed polarizers.

  7. Polarization and hyperfine transitions of metastable ^{129}Xe in discharge cells

    NASA Astrophysics Data System (ADS)

    Xia, T.; Morgan, S. W.; Jau, Y.-Y.; Happer, W.

    2010-03-01

    The polarization and relaxation rates of metastable Xe129 atoms are measured with magnetic resonance spectroscopy, at both microwave frequencies, where ΔF=1 transitions are induced between the sublevels, and at radiofrequencies, corresponding to ΔF=0 transitions. The nuclear spin polarization of the resonant velocity group is measured to be 22±2%. The relaxation of metastable xenon atoms is dominated by depolarizing collisions with ground-state atoms, with lesser contributions from metastability exchange collisions.

  8. Polarized Neutron in Structural Biology Present and Future Outlook

    SciTech Connect

    Zhao, Jinkui; Robertson, Lee; Herwig, Kenneth W; Crabb, Don

    2013-01-01

    Hydrogen has a strong polarization-dependent neutron scattering cross section. This property has been exploited in the study of soft matters, especially biological macromolecules. When a polarized neutron beam is scattered off a polarized hydrogenous sample, the otherwise large hydrogen incoherent cross section is drastically reduced while the coherent signal is significantly increased. Past experiments have demonstrated the potentials and benefits of polarized neutron scattering from soft materials. The main technical challenge of polarized neutron scattering from biological matters lies at sample polarization. Dynamic nuclear polarization is a proven yet rather sophisticated technique. Its complexity is one of the main reasons for the technique's slow adoption. The future of polarized neutron scattering in biology may rest largely in neutron protein crystallography. Polarization of protein crystals is much easier to accomplish, since protein crystals are typically rather small (<<1 mm) and only require small and easy- to-operate polarization apparatuses. In addition, the high resolution nature of neutron protein crystallography means that we will be able to study individual atoms using the polarized neutron scattering technique.

  9. Bulk modulus for polar covalent crystals

    PubMed Central

    Xu, Bo; Wang, Qianqian; Tian, Yongjun

    2013-01-01

    A microscopic empirical model of bulk modulus based on atomic-scale parameters is proposed. These parameters include the bond length, the effective bonded valence electron (EBVE) number, and the coordination number product of two bonded atoms, etc. The estimated bulk moduli from our model are in good agreement with experimental values for various polar covalent crystals including ionic crystals. Our current work sheds lights on the nature of bulk modulus, provides useful clues for design of crystals with low compressibility, and is applicable to complex crystals such as minerals of geophysical importance. PMID:24166098

  10. Atom Skimmers and Atom Lasers Utilizing Them

    NASA Technical Reports Server (NTRS)

    Hulet, Randall; Tollett, Jeff; Franke, Kurt; Moss, Steve; Sackett, Charles; Gerton, Jordan; Ghaffari, Bita; McAlexander, W.; Strecker, K.; Homan, D.

    2005-01-01

    Atom skimmers are devices that act as low-pass velocity filters for atoms in thermal atomic beams. An atom skimmer operating in conjunction with a suitable thermal atomic-beam source (e.g., an oven in which cesium is heated) can serve as a source of slow atoms for a magneto-optical trap or other apparatus in an atomic-physics experiment. Phenomena that are studied in such apparatuses include Bose-Einstein condensation of atomic gases, spectra of trapped atoms, and collisions of slowly moving atoms. An atom skimmer includes a curved, low-thermal-conduction tube that leads from the outlet of a thermal atomic-beam source to the inlet of a magneto-optical trap or other device in which the selected low-velocity atoms are to be used. Permanent rare-earth magnets are placed around the tube in a yoke of high-magnetic-permeability material to establish a quadrupole or octupole magnetic field leading from the source to the trap. The atoms are attracted to the locus of minimum magnetic-field intensity in the middle of the tube, and the gradient of the magnetic field provides centripetal force that guides the atoms around the curve along the axis of the tube. The threshold velocity for guiding is dictated by the gradient of the magnetic field and the radius of curvature of the tube. Atoms moving at lesser velocities are successfully guided; faster atoms strike the tube wall and are lost from the beam.

  11. Pulsed Dynamic Nuclear Polarization with Trityl Radicals.

    PubMed

    Mathies, Guinevere; Jain, Sheetal; Reese, Marcel; Griffin, Robert G

    2016-01-01

    Continuous-wave (CW) dynamic nuclear polarization (DNP) is now established as a method of choice to enhance the sensitivity in a variety of NMR experiments. Nevertheless, there remains a need for the development of more efficient methods to transfer polarization from electrons to nuclei. Of particular interest are pulsed DNP methods because they enable a rapid and efficient polarization transfer that, in contrast with CW DNP methods, is not attenuated at high magnetic fields. Here we report nuclear spin orientation via electron spin-locking (NOVEL) experiments using the polarizing agent trityl OX063 in glycerol/water at a temperature of 80 K and a magnetic field of 0.34 T. (1)H NMR signal enhancements up to 430 are observed, and the buildup of the local polarization occurs in a few hundred nanoseconds. Thus, NOVEL can efficiently dynamically polarize (1)H atoms in a system that is of general interest to the solid-state DNP NMR community. This is a first, important step toward the general application of pulsed DNP at higher fields. PMID:26651876

  12. Device For Viewing Polarized Light

    NASA Technical Reports Server (NTRS)

    Noever, David A.

    1995-01-01

    Technique for detection of polarized light based on observation of scene through two stacked polarizing disks. No need to rotate polarizers to create flicker indicative of polarization. Implemented by relatively simple, lightweight apparatus. Polarization seen as bow-tie rainbow pattern. Advantageous for detecting polarization in variety of meteorological, geological, astronomical, and related applications.

  13. Viewing minerals, atom by atom

    NASA Astrophysics Data System (ADS)

    Maggs, William Ward

    With state-of-the-art technology supported by scissors and bungy cords, Earth scientists are beginning to look at mineral surfaces and mineral-fluid interactions on an atomic scale.The instrument that can provide such a detailed view is the scanning tunneling microscope (STM), which made a great theoretical and practical splash when it was introduced in 1981 by Gerd Binnig and Heinrich Rohrer, physicists at IBM's laboratory in Zurich. They won a Nobel Prize in Physics for their work 5 years later.

  14. Study of a polarized hydrogen ion source with deuterium plasma ionizer

    SciTech Connect

    Belov, A.S.; Derevyankin, G.E.; Dudnikov, V.G.; Klenov, V.S.; Nechaeva, L.P.; Plohinsky, Y.V.; Vasil`ev, G.A.; Yakushev, V.P.

    1995-07-15

    A description of the atomic beam polarized hydrogen ion source developed at the INR in Moscow is given. It is capable of producing polarized 100 {mu}sec long H{sup +} beams with currents up to 6 {mu}A. The beam is 85% polarized and has a normal emittance of 2{pi} mm mrad. Additionally polarized H{sup {minus}} beams have currents up to 200 {mu}A and normalized emittance 2.2 {pi} mm mrad. (AIP)

  15. Consecutive polarizers arrangement producing maximum polarized light intensity

    NASA Astrophysics Data System (ADS)

    Wirjawan, Johannes V. D.

    2016-03-01

    Polarizer mainly functions as a specific filter that blocks or transmits lights of certain polarization. Malus' law predicts the average intensity of polarized light passing a polarizer that transmits certain polarization direction will be proportional to the squared cosine of angle between the two polarization directions. Arranging several polarizers consecutively with various transmission directions will produce various final intensity as well as final polarized direction. Specific arrangement of an arbitrary number (N > 3) of polarizers producing maximum intensity of polarized light will be discussed in this paper. In addition, interesting pattern of maximum values of some trigonometric functions that are difficult to be solved analytically can be obtained from this discussion.

  16. Polarization properties of long-lived stimulated photon echo

    NASA Astrophysics Data System (ADS)

    Reshetov, V. A.; Popov, E. N.

    2015-01-01

    The polarization properties of the long-lived stimulated photon echo formed on the transition ja → jb with the atomic levels degenerate in the projections of the angular momenta are studied theoretically. The two particular transitions ja = 1 → jb = 0 and ja = 1 → jb = 1 with degenerate ground state ja = 1 are discussed. For the transitions ja = 1 → jb = 1 the polarizations and areas of the first (‘write’) and the third (‘read’) excitation pulses are found when the echo polarization faithfully reproduces the arbitrary polarization of the weak (single-photon) second (‘information’) pulse, so that this echo scheme may implement the quantum memory for a single-photon polarization qubit, while for the transitions ja = 1 → jb = 0 it is shown, that the echo polarization differs from that of the second pulse at any conditions.

  17. Plasmonic metasurface for simultaneous detection of polarization and spectrum.

    PubMed

    Pelzman, Charles; Cho, Sang-Yeon

    2016-03-15

    We present a new plasmonic metasurface for simultaneous detection of polarization and spectrum of incident light. The demonstrated metasurface is a rationally designed cluster of artificial atoms that are engineered to exhibit polarization and wavelength-selective optical transmission. The fundamental building block of this structure is periodically coupled subwavelength aperture arrays with different orientations and lattice constants. When integrated with pixelated photodetectors, the metasurface can be used to measure the polarization and spectral information of an optical input. In this Letter, simultaneous detection of the polarization and spectrum of polarized light was experimentally demonstrated by analyzing the transmitted intensity distribution through the metasurface. The demonstrated metasurface offers great potential for many applications, such as polarimetric multispectral imaging and polarization-division multiplexing in optical communications. PMID:26977672

  18. POLARIZED ION SOURCES FOR HIGH ENERGY ACCELERATORS AND COLLIDERS

    SciTech Connect

    ZELENSKI,A.N.

    2000-10-16

    The recent progress in polarized ion source development is reviewed. In dc operation a 1.0 mA polarized H{sup -} ion current is now available from the Optically-Pumped Polarized Ion Source (OPPIS) . In pulsed operation a 10 mA polarized H{sup -} ion current was demonstrated at the TRIUMF pulsed OPPIS test bench and a 3.5 mA peak current was obtained from an Atomic Beam Source (ABS) at the INR Moscow test bench. The possibilities for future improvements with both techniques are discussed. A new OPPIS for RHIC spin physics is described. The OPPIS reliably delivered polarized beam for the polarized run at RHIC. The results obtained with a new pulsed ABS injector for the IUCF Cooler Ring are also discussed.

  19. POLARIZED ION SOURCES FOR HIGH ENERGY ACCELERATORS AND COLLIDERS

    SciTech Connect

    ZELENSKI,A.N.

    2000-10-16

    The recent progress in polarized ion source development is reviewed. In dc operation a 1.0 mA polarized H{sup -} ion current is now available from the Optically-Pumped Polarized Ion Source (OPPIS). In pulsed operation a 10 mA polarized H{sup -} ion current was demonstrated at the TRIUMF pulsed OPPIS test bench and a 3.5 mA peak current was obtained from an Atomic Beam Source (ABS) at the INR Moscow test bench. The possibilities for future improvements with both techniques are discussed. A new OPPIS for RHIC spin physics is described. The OPPIS reliably delivered polarized beam for the polarized run at RHIC. The results obtained with a new pulsed ABS injector for the IUCF Cooler Ring are also discussed.

  20. Spin polarization of the split Kondo state.

    PubMed

    von Bergmann, Kirsten; Ternes, Markus; Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

    2015-02-20

    Spin-resolved scanning tunneling microscopy is employed to quantitatively determine the spin polarization of the magnetic field-split Kondo state. Tunneling conductance spectra of a Kondo-screened magnetic atom are evaluated within a simple model taking into account inelastic tunneling due to spin excitations and two Kondo peaks positioned symmetrically around the Fermi energy. We fit the spin state of the Kondo-screened atom with a spin Hamiltonian independent of the Kondo effect and account for Zeeman splitting of the Kondo peak in the magnetic field. We find that the width and the height of the Kondo peaks scales with the Zeeman energy. Our observations are consistent with full spin polarization of the Kondo peaks, i.e., a majority spin peak below the Fermi energy and a minority spin peak above. PMID:25763966

  1. Interface control of bulk ferroelectric polarization

    PubMed Central

    Yu, P.; Luo, W.; Yi, D.; Zhang, J. X.; Rossell, M. D.; Yang, C.-H.; You, L.; Singh-Bhalla, G.; Yang, S. Y.; He, Q.; Ramasse, Q. M.; Erni, R.; Martin, L. W.; Chu, Y. H.; Pantelides, S. T.; Pennycook, S. J.; Ramesh, R.

    2012-01-01

    The control of material interfaces at the atomic level has led to novel interfacial properties and functionalities. In particular, the study of polar discontinuities at interfaces between complex oxides lies at the frontier of modern condensed matter research. Here we employ a combination of experimental measurements and theoretical calculations to demonstrate the control of a bulk property, namely ferroelectric polarization, of a heteroepitaxial bilayer by precise atomic-scale interface engineering. More specifically, the control is achieved by exploiting the interfacial valence mismatch to influence the electrostatic potential step across the interface, which manifests itself as the biased-voltage in ferroelectric hysteresis loops and determines the ferroelectric state. A broad study of diverse systems comprising different ferroelectrics and conducting perovskite underlayers extends the generality of this phenomenon. PMID:22647612

  2. Automatic Bayesian polarity determination

    NASA Astrophysics Data System (ADS)

    Pugh, D. J.; White, R. S.; Christie, P. A. F.

    2016-07-01

    The polarity of the first motion of a seismic signal from an earthquake is an important constraint in earthquake source inversion. Microseismic events often have low signal-to-noise ratios, which may lead to difficulties estimating the correct first-motion polarities of the arrivals. This paper describes a probabilistic approach to polarity picking that can be both automated and combined with manual picking. This approach includes a quantitative estimate of the uncertainty of the polarity, improving calculation of the polarity probability density function for source inversion. It is sufficiently fast to be incorporated into an automatic processing workflow. When used in source inversion, the results are consistent with those from manual observations. In some cases, they produce a clearer constraint on the range of high-probability source mechanisms, and are better constrained than source mechanisms determined using a uniform probability of an incorrect polarity pick.

  3. Automatic Bayesian polarity determination

    NASA Astrophysics Data System (ADS)

    Pugh, D. J.; White, R. S.; Christie, P. A. F.

    2016-04-01

    The polarity of the first motion of a seismic signal from an earthquake is an important constraint in earthquake source inversion. Microseismic events often have low signal-to-noise ratios, which may lead to difficulties estimating the correct first-motion polarities of the arrivals. This paper describes a probabilistic approach to polarity picking that can be both automated and combined with manual picking. This approach includes a quantitative estimate of the uncertainty of the polarity, improving calculation of the polarity probability density function for source inversion. It is sufficiently fast to be incorporated into an automatic processing workflow. When used in source inversion, the results are consistent with those from manual observations. In some cases, they produce a clearer constraint on the range of high-probability source mechanims, and are better constrained than source mechanisms determined using a uniform probability of an incorrect polarity pick.

  4. A dual polarized antenna system using a meanderline polarizer

    NASA Technical Reports Server (NTRS)

    Burger, H. A.

    1978-01-01

    Certain applications of synthetic aperture radars require transmitting on one linear polarization and receiving on two orthogonal linear polarizations for adequate characterization of the surface. To meet the current need at minimum cost, it was desirable to use two identical horizontally polarized shaped beam antennas and to change the polarization of one of them by a polarization conversion plate. The plate was realized as a four-layer meanderline polarizer designed to convert horizontal polarization to vertical.

  5. Atomic hydrogen cleaning of semiconductor photocathodes

    SciTech Connect

    Sinclair, C.K.; Poelker, B.M.; Price, J.S.

    1997-06-01

    Negative Electron Affinity (NEA) semiconductor photocathodes are widely used for the production of polarized electron beams, and are also useful for the production of high brightness electron beams which can be modulated at very high frequencies. Preparation of an atomically clean semiconductor surface is an essential step in the fabrication of a NEA photocathode. This cleaning step is difficult for certain semiconductors, such as the very thin materials which produce the highest beam polarization, and those which have tightly bound oxides and carbides. Using a small RF dissociation atomic hydrogen source, the authors have reproducibly cleaned GaAs wafers which have been only degreased prior to installation in vacuum. They have consistently prepared very high quantum efficiency photocathodes following atomic hydrogen cleaning. Details of their apparatus and most recent results are presented.

  6. Polarization feedback laser stabilization

    DOEpatents

    Esherick, P.; Owyoung, A.

    1987-09-28

    A system for locking two Nd:YAG laser oscillators includes an optical path for feeding the output of one laser into the other with different polarizations. Elliptical polarization is incorporated into the optical path so that the change in polarization that occurs when the frequencies coincide may be detected to provide a feedback signal to control one laser relative to the other. 4 figs.

  7. Observation of polar vortices in oxide superlattices.

    PubMed

    Yadav, A K; Nelson, C T; Hsu, S L; Hong, Z; Clarkson, J D; Schlepütz, C M; Schlepüetz, C M; Damodaran, A R; Shafer, P; Arenholz, E; Dedon, L R; Chen, D; Vishwanath, A; Minor, A M; Chen, L Q; Scott, J F; Martin, L W; Ramesh, R

    2016-02-11

    The complex interplay of spin, charge, orbital and lattice degrees of freedom provides a plethora of exotic phases and physical phenomena. In recent years, complex spin topologies have emerged as a consequence of the electronic band structure and the interplay between spin and spin-orbit coupling in materials. Here we produce complex topologies of electrical polarization--namely, nanometre-scale vortex-antivortex (that is, clockwise-anticlockwise) arrays that are reminiscent of rotational spin topologies--by making use of the competition between charge, orbital and lattice degrees of freedom in superlattices of alternating lead titanate and strontium titanate layers. Atomic-scale mapping of the polar atomic displacements by scanning transmission electron microscopy reveals the presence of long-range ordered vortex-antivortex arrays that exhibit nearly continuous polarization rotation. Phase-field modelling confirms that the vortex array is the low-energy state for a range of superlattice periods. Within this range, the large gradient energy from the vortex structure is counterbalanced by the corresponding large reduction in overall electrostatic energy (which would otherwise arise from polar discontinuities at the lead titanate/strontium titanate interfaces) and the elastic energy associated with epitaxial constraints and domain formation. These observations have implications for the creation of new states of matter (such as dipolar skyrmions, hedgehog states) and associated phenomena in ferroic materials, such as electrically controllable chirality. PMID:26814971

  8. Asymptotes in Polar Coordinates.

    ERIC Educational Resources Information Center

    Fay, Temple H.

    1986-01-01

    An old way to determine asymptotes for curves described in polar coordinates is presented. Practice in solving trigonometric equations, in differentiation, and in calculating limits is involved. (MNS)

  9. Polarization at SLC

    SciTech Connect

    Swartz, M.L.

    1988-07-01

    The SLAC Linear Collider has been designed to readily accommodate polarized electron beams. Considerable effort has been made to implement a polarized source, a spin rotation system, and a system to monitor the beam polarization. Nearly all major components have been fabricated. At the current time, several source and polarimeter components have been installed. The installation and commissioning of the entire system will take place during available machine shutdown periods as the commissioning of SLC progresses. It is expected that a beam polarization of 45% will be achieved with no loss in luminosity. 13 refs., 15 figs.

  10. Polarization In Remote Sensing

    NASA Astrophysics Data System (ADS)

    Egan, Walter G.

    1988-06-01

    Various aspects of polarization in remote sensing are presented including mathematical treatments and selected experimental observations. The observations are of the percent polarization from Haleakala volcanic ash, basalt powder, rhyolytic oumice. rose quartz, niccolite, ilmenite, black oak leaves. dried red pine needles, a New Haven red pine stand, moist soil, the sky above Mauna Loa Observatory, the sky above Long Island in summer and winter, and cirrus clouds. Also, space based shuttle photographic observations of polarization are described. Instrumental polarization from a Cassegrainian telescope is described as well as the design of an imaging soectropolarimeter for remote sensing. A list is presented of twelve polarimetric properties associated with remote sensing.

  11. Polarized Line Formation with Lower-level Polarization and Partial Frequency Redistribution

    NASA Astrophysics Data System (ADS)

    Supriya, H. D.; Sampoorna, M.; Nagendra, K. N.; Stenflo, J. O.; Ravindra, B.

    2016-09-01

    In the well-established theories of polarized line formation with partial frequency redistribution (PRD) for a two-level and two-term atom, it is generally assumed that the lower level of the scattering transition is unpolarized. However, the existence of unexplained spectral features in some lines of the Second Solar Spectrum points toward a need to relax this assumption. There exists a density matrix theory that accounts for the polarization of all the atomic levels, but it is based on the flat-spectrum approximation (corresponding to complete frequency redistribution). In the present paper we propose a numerical algorithm to solve the problem of polarized line formation in magnetized media, which includes both the effects of PRD and the lower level polarization (LLP) for a two-level atom. First we derive a collisionless redistribution matrix that includes the combined effects of the PRD and the LLP. We then solve the relevant transfer equation using a two-stage approach. For illustration purposes, we consider two case studies in the non-magnetic regime, namely, the J a = 1, J b = 0 and J a = J b = 1, where J a and J b represent the total angular momentum quantum numbers of the lower and upper states, respectively. Our studies show that the effects of LLP are significant only in the line core. This leads us to propose a simplified numerical approach to solve the concerned radiative transfer problem.

  12. Optically-pumped spin-exchange polarized electron source

    NASA Astrophysics Data System (ADS)

    Pirbhai, Munir Hussein

    Polarized electron beams are an indispensable probe of spin-dependent phenomena in fields of atomic and molecular physics, magnetism and biophysics. While their uses have become widespread, the standard source based on negative electron affinity gallium arsenide (GaAs) remains technically complicated. This has hindered progress on many experiments involving spin-polarized electrons, especially those using target gas loads, which tend to adversely affect the performance of GaAs sources. A robust system based on an alternative way to make polarized electron beams has been devised in this study, which builds on previous work done in our lab. It involves spin-exchange collisions between free, unpolarized electrons and oriented rubidium atoms in the presence of a quenching gas. This system has less stringent vacuum requirements than those of GaAs sources, and is capable of operating in background pressures of ~1mTorr. Beams with ~24% polarization and 4μA of current have been recorded, which is comparable to the performance obtained with the earlier version built in our lab. The present system is however not as unstable as in the previous work, and has the potential to be developed into a "turn-key" source of polarized electron beams. It has also allowed us to undertake a study to find factors which affect the beam polarization in this scheme of producing polarized electrons. Such knowledge will help us to design better optically-pumped spin-exchange polarized electron sources.

  13. Dynamical manipulation of electromagnetic polarization using anisotropic meta-mirror.

    PubMed

    Cui, Jianhua; Huang, Cheng; Pan, Wenbo; Pu, Mingbo; Guo, Yinghui; Luo, Xiangang

    2016-01-01

    Polarization control of electromagnetic wave is very important in many fields. Here, we propose an active meta-mirror to dynamically manipulate electromagnetic polarization state at a broad band. This meta-mirror is composed of a double-layered metallic pattern backed by a metallic flat plate, and the active elements of PIN diodes are integrated into the meta-atom to control the reflection phase difference between two orthogonal polarization modes. Through switching the operating state of the PIN diodes, the meta-mirror is expected to achieve three polarization states which are left-handed, right-handed circular polarizations and linear polarization, respectively. We fabricated this active meta-mirror and validated its polarization conversion performance by measurement. The linearly polarized incident wave can be dynamically converted to right-handed or left-handed circular polarization in the frequency range between 3.4 and 8.8 GHz with the average loss of 1 dB. Furthermore, it also can keep its initial linear polarization state. PMID:27469028

  14. Dynamical manipulation of electromagnetic polarization using anisotropic meta-mirror

    NASA Astrophysics Data System (ADS)

    Cui, Jianhua; Huang, Cheng; Pan, Wenbo; Pu, Mingbo; Guo, Yinghui; Luo, Xiangang

    2016-07-01

    Polarization control of electromagnetic wave is very important in many fields. Here, we propose an active meta-mirror to dynamically manipulate electromagnetic polarization state at a broad band. This meta-mirror is composed of a double-layered metallic pattern backed by a metallic flat plate, and the active elements of PIN diodes are integrated into the meta-atom to control the reflection phase difference between two orthogonal polarization modes. Through switching the operating state of the PIN diodes, the meta-mirror is expected to achieve three polarization states which are left-handed, right-handed circular polarizations and linear polarization, respectively. We fabricated this active meta-mirror and validated its polarization conversion performance by measurement. The linearly polarized incident wave can be dynamically converted to right-handed or left-handed circular polarization in the frequency range between 3.4 and 8.8 GHz with the average loss of 1 dB. Furthermore, it also can keep its initial linear polarization state.

  15. Dynamical manipulation of electromagnetic polarization using anisotropic meta-mirror

    PubMed Central

    Cui, Jianhua; Huang, Cheng; Pan, Wenbo; Pu, Mingbo; Guo, Yinghui; Luo, Xiangang

    2016-01-01

    Polarization control of electromagnetic wave is very important in many fields. Here, we propose an active meta-mirror to dynamically manipulate electromagnetic polarization state at a broad band. This meta-mirror is composed of a double-layered metallic pattern backed by a metallic flat plate, and the active elements of PIN diodes are integrated into the meta-atom to control the reflection phase difference between two orthogonal polarization modes. Through switching the operating state of the PIN diodes, the meta-mirror is expected to achieve three polarization states which are left-handed, right-handed circular polarizations and linear polarization, respectively. We fabricated this active meta-mirror and validated its polarization conversion performance by measurement. The linearly polarized incident wave can be dynamically converted to right-handed or left-handed circular polarization in the frequency range between 3.4 and 8.8 GHz with the average loss of 1 dB. Furthermore, it also can keep its initial linear polarization state. PMID:27469028

  16. Atomic displacements in ferroelectric trigonal and orthorhombic boracite structures

    USGS Publications Warehouse

    Dowty, Eric; Clark, J.R.

    1972-01-01

    New crystal-structure refinements of Pca21 boracite, Mg3ClB7O13, and R??{lunate}c ericaite, Fe2.4Mg0.6ClB7O13, show that some boron and oxygen atoms are involved in the 'ferro' transitions as well as the metal and halogen atoms. The atomic displacements associated with the polarity changes are as large as 0.6A??. ?? 1972.

  17. RHIC Polarized proton operation

    SciTech Connect

    Huang, H.; Ahrens, L.; Alekseev, I.G.; Aschenauer, E.; Atoian, G.; Bai, M.; Bazilevsky, A.; Blaskiewicz, M.; Brennan, J.M.; Brown, K.A.; Bruno, D.; Connolly, R.; Dion, A.; D'Ottavio, T.; Drees, K.A.; Fischer, W.; Gardner, C.; Glenn, J.W.; Gu, X.; Harvey, M.; Hayes, T.; Hoff, L.; Hulsart, R.L.; Laster, J.; Liu, C.; Luo, Y.; MacKay, W.W.; Makdisi, Y.; Marr, G.J.; Marusic, A.; Meot, F.; Mernick, K.; Michnoff, R,; Minty, M.; Montag, C.; Morris, J.; Nemesure, S.; Poblaguev, A.; Ptitsyn, V.; Ranjibar, V.; Robert-Demolaize, G.; Roser, T.; J.; Severino, F.; Schmidke, B.; Schoefer, V.; Severino, F.; Smirnov, D.; Smith, K.; Steski, D.; Svirida, D.; Tepikian, S.; Trbojevic, D.; Tsoupas, N.; Tuozzolo, J. Wang, G.; Wilinski, M.; Yip, K.; Zaltsman, A.; Zelenski, A.; Zeno, K.; Zhang, S.Y.

    2011-03-28

    The Relativistic Heavy Ion Collider (RHIC) operation as the polarized proton collider presents unique challenges since both luminosity(L) and spin polarization(P) are important. With longitudinally polarized beams at the experiments, the figure of merit is LP{sup 4}. A lot of upgrades and modifications have been made since last polarized proton operation. A 9 MHz rf system is installed to improve longitudinal match at injection and to increase luminosity. The beam dump was upgraded to increase bunch intensity. A vertical survey of RHIC was performed before the run to get better magnet alignment. The orbit control is also improved this year. Additional efforts are put in to improve source polarization and AGS polarization transfer efficiency. To preserve polarization on the ramp, a new working point is chosen such that the vertical tune is near a third order resonance. The overview of the changes and the operation results are presented in this paper. Siberian snakes are essential tools to preserve polarization when accelerating polarized beams to higher energy. At the same time, the higher order resonances still can cause polarization loss. As seen in RHIC, the betatron tune has to be carefully set and maintained on the ramp and during the store to avoid polarization loss. In addition, the orbit control is also critical to preserve polarization. The higher polarization during this run comes from several improvements over last run. First we have a much better orbit on the ramp. The orbit feedback brings down the vertical rms orbit error to 0.1mm, much better than the 0.5mm last run. With correct BPM offset and vertical realignment, this rms orbit error is indeed small. Second, the jump quads in the AGS improved input polarization for RHIC. Third, the vertical tune was pushed further away from 7/10 snake resonance. The tune feedback maintained the tune at the desired value through the ramp. To calibrate the analyzing power of RHIC polarimeters at any energy above

  18. First principles calculation of the structural, electronic, and magnetic properties of Au-Pd atomic chains

    SciTech Connect

    Dave, Mudra R.; Sharma, A. C.

    2015-06-24

    The structural, electronic and magnetic properties of free standing Au-Pd bimetallic atomic chain is studied using ab-initio method. It is found that electronic and magnetic properties of chains depend on position of atoms and number of atoms. Spin polarization factor for different atomic configuration of atomic chain is calculated predicting a half metallic behavior. It suggests a total spin polarised transport in these chains.

  19. Polarized electron scattering, new physics and dark parity violation

    SciTech Connect

    Marciano, William J.

    2013-11-07

    'New Physics' sensitivities of polarized electron scattering asymmetries, atomic parity violation, m{sub W} and sin{sup 2} θ{sub W} (Z pole measurements) are compared. The utility of low Q{sup 2} polarized electron scattering for probing parity violating 'dark boson' effects is discussed. A possible determination of the weak charge Q{sub w}({sup 12}C) to about ±0.3% via elastic e-Carbon scattering is advocated.

  20. Laser-driven polarized hydrogen and deuterium internal targets

    SciTech Connect

    Jones, C.E.; Fedchak, J.A.; Kowalczyk, R.S.

    1995-08-01

    After completing comprehensive tests of the performance of the source with both hydrogen and deuterium gas, we began tests of a realistic polarized deuterium internal target. These tests involve characterizing the atomic polarization and dissociation fraction of atoms in a storage cell as a function of flow and magnetic field, and making direct measurements of the average nuclear tensor polarization of deuterium atoms in the storage cell. Transfer of polarization from the atomic electron to the nucleus as a result of D-D spin-exchange collisions was observed in deuterium, verifying calculations suggesting that high vector polarization in both hydrogen and deuterium can be obtained in a gas in spin temperature equilibrium without inducing RF transitions between the magnetic substates. In order to improve the durability of the system, the source glassware was redesigned to simplify construction and installation and eliminate stress points that led to frequent breakage. Improvements made to the nuclear polarimeter, which used the low energy {sup 3}H(d,n){sup 4}He reaction to analyze the tensor polarization of the deuterium, included installing acceleration lenses constructed of wire mesh to improve pumping conductance, construction of a new holding field coil, and elimination of the Wien filter from the setup. These changes substantially simplified operation of the polarimeter and should have reduced depolarization in collisions with the wall. However, when a number of tests failed to show an improvement of the nuclear polarization, it was discovered that extended operation of the system with a section of teflon as a getter for potassium caused the dissociation fraction to decline with time under realistic operating conditions, suggesting that teflon may not be a suitable material to eliminate potassium from the target. We are replacing the teflon surfaces with drifilm-coated ones and plan to continue tests of the polarized internal target in this configuration.

  1. Development of a Polarized 3He Ion Source for RHIC

    SciTech Connect

    Milner, Richard G.

    2013-01-15

    The goal of the project was to design and construct a source of polarized 3He atoms for injection into EBIS. This is the initial step in producing polarized 3He beams in RHIC in collaboration with physicists from Columbia University and Brookhaven National Laboratory. These beams can be used to probe the spin structure of the neutron in the existing RHIC complex as well as to measure precisely the Bjorken Sum Rule at a future eRHIC electron-ion collider.

  2. The Polar Insulation Investigation

    ERIC Educational Resources Information Center

    Urban-Rich, Juanita

    2006-01-01

    In this article, the author developed an activity called "The Polar Insulation Investigation." This activity builds on students' natural interest in "things polar" and introduces them to animal adaptations in a unique way. The aim of the exploration is to determine the role of animal coverings (e.g., blubber, fur, and feathers) and to see which is…

  3. Our Polar Past

    ERIC Educational Resources Information Center

    Clary, Renee; Wandersee, James

    2009-01-01

    The study of polar exploration is fascinating and offers students insights into the history, culture, and politics that affect the developing sciences at the farthest ends of Earth. Therefore, the authors think there is value in incorporating polar exploration accounts within modern science classrooms, and so they conducted research to test their…

  4. Polar Science Is Cool!

    ERIC Educational Resources Information Center

    Weeks, Sophie

    2012-01-01

    Children are fascinated by the fact that polar scientists do research in extremely cold and dangerous places. In the Arctic they might be viewed as lunch by a polar bear. In the Antarctic, they could lose toes and fingers to frostbite and the wind is so fast it can rip skin off. They camp on ice in continuous daylight, weeks from any form of…

  5. Polarized Light: Three Demonstrations.

    ERIC Educational Resources Information Center

    Goehmann, Ruth; Welty, Scott

    1984-01-01

    Describes three demonstrations used in the Chicago Museum of Science and Industry polarized light show. The procedures employed are suitable for the classroom by using smaller polarizers and an overhead projector. Topic areas include properties of cellophane tape, nondisappearing arrows, and rope through a picket fence. (JN)

  6. Mechanism of lunar polarization.

    PubMed

    Hopfield, J J

    1966-03-18

    A theoretical model to explain the negative polarization of moonlight at small lunar phase angles is developed. The model is based on the polarization of light in the diffraction region bordering the geometric shadow of an opaque dielectric obstacle. PMID:17817298

  7. Production of intense beams of polarized negative hydrogen ions by double charge exchange in alkali vapour

    NASA Astrophysics Data System (ADS)

    Gruëbler, W.; Schmelzbach, P. A.

    1983-07-01

    The intensity of the polarized negative hydrogen ion beam of the ETHZ atomic beam polarized ion source has been substantially improved by a new double charge exchange device. Increasing the diameter of the charge exchange canal to 1.4 cm results in a beam output of the source of 6 μA of polarized negative hydrogen ions. Further improvements of the charge exchanger are proposed and discussed. With an updated design of the atomic beam apparatus, beams of 0.5 mA polarized negative hydrogen ions may be obtained from such a source.

  8. Excess optical quantum noise in atomic sensors

    NASA Astrophysics Data System (ADS)

    Novikova, Irina; Mikhailov, Eugeniy; Xiao, Yanhong

    2015-05-01

    Enhanced nonlinear optical response of a coherent atomic medium is the basis for many atomic sensors, and their performance is ultimately limited by the quantum fluctuations of the optical read-out. Here we demonstrate that off-resonant interactions can significantly modify the quantum noise of the optical field, even when their effect on the mean signal is negligible. We illustrate this concept by using an atomic magnetometer based on the nonlinear Faraday effect: the rotation of the light polarization is mainly determined by the resonant light-induced spin alignment, which alone does not change the photon statistics of the optical probe. Yet, we found that the minimum noise of output polarization rotation measurements is above the expected shot noise limit. This excess quantum noise is due to off-resonant coupling and grows with atomic density. We also show that the detection scheme can be modified to reduce the measured quantum noise (even below the shot-noise limit) but only at the expense of the reduced rotational sensitivity. These results show the existence of previously unnoticed factors in fundamental limitations in atomic magnetometry and could have impacts in many other atom-light based precision measurements. We acknowledge the support from AFOSR (grant FA9550-13-1-0098), NSF (grant PHY-1308281), NBRPC(973 Program Grant 2012CB921604 and 2011CB921604), and NNSFC (Grants No. 11322436).

  9. Polarization and polarization fatigue in ferroelectrics

    NASA Astrophysics Data System (ADS)

    Du, Xiaofeng

    This thesis addresses some fundamental issues in ferroelectricity and its applications through a computational and experimental effort. It focuses on a variety of perovskite-type ferroelectric oxides and investigates the physical basis for spontaneous polarization, domain wall dynamics, and texture development in thin film applications. The dipole-dipole interactions between ionic species in perovskite-type materials have been calculated to determine the local field and the lattice instability. Different ferroelectric and anti-ferroelectric polarization transitions can be realized by taking into account the structure distortion of the parent perovskites. We find the local field is enhanced by short range disorder and its nature varies from disorder to disorder, causing polarization transitions in non-(100) directions. The molecular field theory has also been extended to layered perovskites, which favors in-plane polarization over c-polarization. These theoretical predictions are in agreement with the experimental observations of various perovskites and layered perovskites in both single crystal and thin film forms. Domain switching in PZT has been studied by probing the frequency dependency of polarization hysteresis. A picture of thermally activated domain wall movement is established from the frequency spectra of coercive field. The field dependence of domain wall bulging and the nature of the binding between pinning obstacles and the walls are inferred from such a study. Consistent with this picture, polarization fatigue can be defined as a process of increasing the resistance from pinning defects to domain wall motion. The chemical species that act as pinning defects have been identified through model experiments that control carrier injection, electrode interfaces, and film compositions. Based on these observations, a methodology is proposed to evaluate and predict the fatigue damage of both PZT and layered perovskite thin films. Processing of layered

  10. Parallel Polarization State Generation

    PubMed Central

    She, Alan; Capasso, Federico

    2016-01-01

    The control of polarization, an essential property of light, is of wide scientific and technological interest. The general problem of generating arbitrary time-varying states of polarization (SOP) has always been mathematically formulated by a series of linear transformations, i.e. a product of matrices, imposing a serial architecture. Here we show a parallel architecture described by a sum of matrices. The theory is experimentally demonstrated by modulating spatially-separated polarization components of a laser using a digital micromirror device that are subsequently beam combined. This method greatly expands the parameter space for engineering devices that control polarization. Consequently, performance characteristics, such as speed, stability, and spectral range, are entirely dictated by the technologies of optical intensity modulation, including absorption, reflection, emission, and scattering. This opens up important prospects for polarization state generation (PSG) with unique performance characteristics with applications in spectroscopic ellipsometry, spectropolarimetry, communications, imaging, and security. PMID:27184813

  11. Polarization of clouds

    NASA Astrophysics Data System (ADS)

    Goloub, Philippe; Herman, Maurice; Parol, Frederic

    1995-12-01

    This paper reports the main results concerning polarization by clouds derived from POLDER (polarization and directionality of earth's reflectances) airborne version. These results tend to confirm the high information content in the polarization (phase, altimetry). The preliminary results of EUCREX'94 (European Cloud Radiation Experiment) evidenced the drastically different polarized signatures for ice crystals and water droplets. Here we report systematic and statistically significative observations over the whole EUCREX data set. The results show that the cirrus exhibit their own signature. Preliminary observations performed during CLEOPATRA'91 (Cloud Experiment Ober Pfaffenhofen And Transport) and EUCREX'94 campaigns have shown the feasibility of cloud altimetry using spectral information (443 nm and 865 nm) of the polarized light over liquid water droplets clouds. Altimetry technique has been generalized on ASTEX-SOFIA'92 and EUCREX'94 data sets. All these results are presented and discussed in this paper.

  12. Precision Polarization of Neutrons

    NASA Astrophysics Data System (ADS)

    Martin, Elise; Barron-Palos, Libertad; Couture, Aaron; Crawford, Christopher; Chupp, Tim; Danagoulian, Areg; Estes, Mary; Hona, Binita; Jones, Gordon; Klein, Andi; Penttila, Seppo; Sharma, Monisha; Wilburn, Scott

    2009-05-01

    Determining polarization of a cold neutron beam to high precision is required for the next generation neutron decay correlation experiments at the SNS, such as the proposed abBA and PANDA experiments. Precision polarimetry measurements were conducted at Los Alamos National Laboratory with the goal of determining the beam polarization to the level of 10-3 or better. The cold neutrons from FP12 were polarized using optically polarized ^3He gas as a spin filter, which has a highly spin-dependent absorption cross section. A second ^ 3He spin filter was used to analyze the neutron polarization after passing through a resonant RF spin rotator. A discussion of the experiment and results will be given.

  13. Parallel Polarization State Generation

    NASA Astrophysics Data System (ADS)

    She, Alan; Capasso, Federico

    2016-05-01

    The control of polarization, an essential property of light, is of wide scientific and technological interest. The general problem of generating arbitrary time-varying states of polarization (SOP) has always been mathematically formulated by a series of linear transformations, i.e. a product of matrices, imposing a serial architecture. Here we show a parallel architecture described by a sum of matrices. The theory is experimentally demonstrated by modulating spatially-separated polarization components of a laser using a digital micromirror device that are subsequently beam combined. This method greatly expands the parameter space for engineering devices that control polarization. Consequently, performance characteristics, such as speed, stability, and spectral range, are entirely dictated by the technologies of optical intensity modulation, including absorption, reflection, emission, and scattering. This opens up important prospects for polarization state generation (PSG) with unique performance characteristics with applications in spectroscopic ellipsometry, spectropolarimetry, communications, imaging, and security.

  14. Parallel Polarization State Generation.

    PubMed

    She, Alan; Capasso, Federico

    2016-01-01

    The control of polarization, an essential property of light, is of wide scientific and technological interest. The general problem of generating arbitrary time-varying states of polarization (SOP) has always been mathematically formulated by a series of linear transformations, i.e. a product of matrices, imposing a serial architecture. Here we show a parallel architecture described by a sum of matrices. The theory is experimentally demonstrated by modulating spatially-separated polarization components of a laser using a digital micromirror device that are subsequently beam combined. This method greatly expands the parameter space for engineering devices that control polarization. Consequently, performance characteristics, such as speed, stability, and spectral range, are entirely dictated by the technologies of optical intensity modulation, including absorption, reflection, emission, and scattering. This opens up important prospects for polarization state generation (PSG) with unique performance characteristics with applications in spectroscopic ellipsometry, spectropolarimetry, communications, imaging, and security. PMID:27184813

  15. Cell polarity: mechanochemical patterning.

    PubMed

    Goehring, Nathan W; Grill, Stephan W

    2013-02-01

    Nearly every cell type exhibits some form of polarity, yet the molecular mechanisms vary widely. Here we examine what we term 'chemical systems' where cell polarization arises through biochemical interactions in signaling pathways, 'mechanical systems' where cells polarize due to forces, stresses and transport, and 'mechanochemical systems' where polarization results from interplay between mechanics and chemical signaling. To reveal potentially unifying principles, we discuss mathematical conceptualizations of several prototypical examples. We suggest that the concept of local activation and global inhibition - originally developed to explain spatial patterning in reaction-diffusion systems - provides a framework for understanding many cases of cell polarity. Importantly, we find that the core ingredients in this framework - symmetry breaking, self-amplifying feedback, and long-range inhibition - involve processes that can be chemical, mechanical, or even mechanochemical in nature. PMID:23182746

  16. Investigation of xenon metastable atoms

    NASA Astrophysics Data System (ADS)

    Xia, Tian; Jau, Yuan-Yu; Happer, William

    2007-06-01

    The electron configuration of a xenon atom in its metastable state consists of tightly bound core electrons with a single missing electron in the 5P shell, and a loosely bound ``valence electron'' in the 6S shell. For our current work, we have been using pyrex cells with internal tungsten electrodes, filled with isotopically enriched Xe129 gas. Ti-sapphire laser is used to pump the metastable atom from 6S2 to 6P2 and 6P3 at 823nm and 882nm respectively. The absorption spectrum is able to resolve the hyperfine structure of Xe129 in 6S2, 6P2 and 6P3 state. The hyperfine coefficients for 6S2, 6P2 agree with previously reported measurements. And the hyperfine coefficient for 6P3 state has not been reported before. If the pumping wavelength is locked at any one of the hyperfine transitions of Xenon129 atom, zero-field magnetic resonances of metastable Xenon atoms could be observed by pumping with circularly polarized laser beam. Since relaxation between magnetic sublevels is very fast due to the big depolarization collisional cross section, the linewidth of the magnetic resonant signal is broad.

  17. Molecular content of polar-ring galaxies

    NASA Astrophysics Data System (ADS)

    Combes, F.; Moiseev, A.; Reshetnikov, V.

    2013-06-01

    We have searched for CO lines in a sample of 21 new morphologically determined polar-ring galaxies (of which nine are kinematically confirmed), obtained from a wide search in the Galaxy Zoo project by Moiseev and collaborators. Polar-ring galaxies (PRGs) are a unique class of objects, tracing special episodes in the galaxy mass assembly: they can be formed through galaxy interaction and merging, but also through accretion from cosmic filaments. Furthermore, they enable the study of dark matter haloes in three dimensions. The polar ring itself is a sub-system rich in gas, where molecular gas is expected, and new stars are formed. Among the sample of 21 PRGs, we have detected five CO-rich systems, that can now be followed up with higher spatial resolution. Their average molecular mass is 9.4 × 109M⊙, and their average gas fraction is 27% of their baryonic mass, with a range from 15 to 43%, implying that they have just accreted a large amount of gas. The position of the detected objects in the velocity-magnitude diagram is offset from the Tully-Fisher relation of normal spirals, as was already found for PRGs. This work is part of our multi-wavelength project to determine the detailed morphology and dynamics of PRGs, test through numerical models their formation scenario, and deduce their dark matter content and 3D-shape. Based on observations carried out with the IRAM 30 m telescope. IRAM is supported by INSU/CNRS (France), MPG (Germany), and IGN (Spain).Spectra of detections are available at the CDS via anonymous ftp to cdsarc.u-strasbg.fr (ftp://130.79.128.5">130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/554/A11

  18. Observation of Polar Vortices in Oxide Superlattices

    NASA Astrophysics Data System (ADS)

    Ramesh, R.

    The complex interplay of spin, charge, orbital, and lattice degrees of freedom has provided for a plethora of exotic phase and physical phenomena. Among these, in recent years, topological states of matter and spin textures have emerged as fascinating consequences of the electronic band structure and the interplay between spin and spin-orbit coupling in materials. In this work, we leverage the competition between charge, orbital, and lattice degrees of freedom in superlattices of PbTiO3/SrTiO3 to produce complex, vortex-antivortex pairs (that exhibit smoothly varying ferroelectric polarization with a 10 nm periodicity) that are reminiscent of topological features such as skyrmions and merons. Using a combination of advanced layer-by-layer growth techniques, atomic-resolution mapping of structure and local polar distortions using scanning-transmission electron microscopy, and phase-field modeling approaches we present a comprehensive picture of the nature of the varying polarization profile in such vortex states. The continuous rotation of the polar state into the vortex structures is thought to occur from an interplay of polar discontinuities at the PbTiO3/SrTiO3 interface (where), the phase transformation strain and gradient energy in the PbTiO3 layer, and the strain imposed by the substrate. Finally, the implications of these observations are discussed as they pertain to producing new states of matter and phenomena in ferroic materials.

  19. Scattering of twisted relativistic electrons by atoms

    NASA Astrophysics Data System (ADS)

    Serbo, V.; Ivanov, I. P.; Fritzsche, S.; Seipt, D.; Surzhykov, A.

    2015-07-01

    The Mott scattering of high-energetic twisted electrons by atoms is investigated within the framework of the first Born approximation and Dirac's relativistic equation. Special emphasis is placed on the angular distribution and longitudinal polarization of the scattered electrons. In order to evaluate these angular and polarization properties we consider two experimental setups in which the twisted electron beam collides with either a single well-localized atom or macroscopic atomic target. Detailed relativistic calculations have been performed for both setups and for the electrons with kinetic energy from 10 to 1000 keV. The results of these calculations indicate that the emission pattern and polarization of outgoing electrons differ significantly from the scattering of plane-wave electrons and can be very sensitive to the parameters of the incident twisted beam. In particular, it is shown that the angular- and polarization-sensitive Mott measurements may reveal valuable information about both the transverse and longitudinal components of the linear momentum and the projection of the total angular momentum of twisted electron states. Thus, the Mott scattering emerges as a diagnostic tool for the relativistic vortex beams.

  20. Dressed spin of polarized {sup 3}He in a cell

    SciTech Connect

    Chu, P.-H.; Esler, A. M.; Peng, J. C.; Beck, D. H.; Chandler, D. E.; Clayton, S.; Williamson, S.; Yoder, J.; Hu, B.-Z.; Ngan, S. Y.; Sham, C. H.; So, L. H.

    2011-08-15

    We report a measurement of the modification of the effective precession frequency of polarized {sup 3}He atoms in response to a dressing field in a room-temperature cell. The {sup 3}He atoms were polarized using the metastability spin-exchange method. An oscillating dressing field was then applied perpendicular to the constant magnetic field. Modification of the {sup 3}He effective precession frequency was observed over a broad range of the amplitude and frequency of the dressing field. The observed effects are compared with calculations based on quantum optics formalism.

  1. Dressed spin of polarized 3He in a cell

    NASA Astrophysics Data System (ADS)

    Chu, P.-H.; Esler, A. M.; Peng, J. C.; Beck, D. H.; Chandler, D. E.; Clayton, S.; Hu, B.-Z.; Ngan, S. Y.; Sham, C. H.; So, L. H.; Williamson, S.; Yoder, J.

    2011-08-01

    We report a measurement of the modification of the effective precession frequency of polarized 3He atoms in response to a dressing field in a room-temperature cell. The 3He atoms were polarized using the metastability spin-exchange method. An oscillating dressing field was then applied perpendicular to the constant magnetic field. Modification of the 3He effective precession frequency was observed over a broad range of the amplitude and frequency of the dressing field. The observed effects are compared with calculations based on quantum optics formalism.

  2. Switchable polarization in an unzipped graphene oxide monolayer.

    PubMed

    Noor-A-Alam, Mohammad; Shin, Young-Han

    2016-08-14

    Ferroelectricity in low-dimensional oxide materials is generally suppressed at the scale of a few nanometers, and has attracted considerable attention from both fundamental and technological aspects. Graphene is one of the thinnest materials (one atom thick). Therefore, engineering switchable polarization in non-polar pristine graphene could potentially lead to two-dimensional (2D) ferroelectric materials. In the present study, based on density functional theory, we show that an unzipped graphene oxide (UGO) monolayer can exhibit switchable polarization due to its foldable bonds between the oxygen atom and two carbon atoms underneath the oxygen. We find that a free standing UGO monolayer exhibits antiferroelectric switchable polarization. A UGO monolayer can be obtained as an intermediate product during the chemical exfoliation process of graphene. Interestingly, despite its dimensionality, our estimated polarization in a UGO monolayer is comparable to that in bulk ferroelectric materials (e.g., ferroelectric polymers). Our calculations could help realize antiferroelectric switchable polarization in 2D materials, which could find various potential applications in nanoscale devices such as sensors, actuators, and capacitors with high energy-storage density. PMID:27401944

  3. "Bohr's Atomic Model."

    ERIC Educational Resources Information Center

    Willden, Jeff

    2001-01-01

    "Bohr's Atomic Model" is a small interactive multimedia program that introduces the viewer to a simplified model of the atom. This interactive simulation lets students build an atom using an atomic construction set. The underlying design methodology for "Bohr's Atomic Model" is model-centered instruction, which means the central model of the…

  4. Multipoint Energetic Neutral Atom Studies with Polar, Geotail, and Tiros

    NASA Technical Reports Server (NTRS)

    Spence, Harlan E.

    2001-01-01

    This final report describes the efforts accomplished during the grant's period of performance, covering the period of 15 January 1999 to 14 January 2001, of a NASA ISTP/SolarMax Extended Science Program grant. We have completed many of the goals set forth in the proposed research objectives and our efforts in this research area continue in a related grant from NASA. Studies have been published and papers are being written, and numerous invited and contributed presentations of these studies have been presented at national and international meetings during the performance period.

  5. TOPICAL REVIEW: Theory and applications of atomic and ionic polarizabilities

    NASA Astrophysics Data System (ADS)

    Mitroy, J.; Safronova, M. S.; Clark, Charles W.

    2010-10-01

    Atomic polarization phenomena impinge upon a number of areas and processes in physics. The dielectric constant and refractive index of any gas are examples of macroscopic properties that are largely determined by the dipole polarizability. When it comes to microscopic phenomena, the existence of alkaline-earth anions and the recently discovered ability of positrons to bind to many atoms are predominantly due to the polarization interaction. An imperfect knowledge of atomic polarizabilities is presently looming as the largest source of uncertainty in the new generation of optical frequency standards. Accurate polarizabilities for the group I and II atoms and ions of the periodic table have recently become available by a variety of techniques. These include refined many-body perturbation theory and coupled-cluster calculations sometimes combined with precise experimental data for selected transitions, microwave spectroscopy of Rydberg atoms and ions, refractive index measurements in microwave cavities, ab initio calculations of atomic structures using explicitly correlated wavefunctions, interferometry with atom beams and velocity changes of laser cooled atoms induced by an electric field. This review examines existing theoretical methods of determining atomic and ionic polarizabilities, and discusses their relevance to various applications with particular emphasis on cold-atom physics and the metrology of atomic frequency standards.

  6. Interplanetary magnetic sector polarity inferred from polar geomagnetic field observations

    NASA Technical Reports Server (NTRS)

    Friis-Christensen, E.; Lassen, K.; Wilcox, J. M.; Gonzalez, W.; Colburn, D. S.

    1971-01-01

    In order to infer the interplanetary sector polarity from polar geomagnetic field diurnal variations, measurements were carried out at Godhavn and Thule (Denmark) Geomagnetic Observatories. The inferred interplanetary sector polarity was compared with the polarity observed at the same time by Explorer 33 and 35 magnetometers. It is shown that the polarity (toward or away from the sun) of the interplanetary magnetic field can be reliably inferred from observations of the polar cap geomagnetic fields.

  7. Neutron Polarizers Based on Polarized 3He

    SciTech Connect

    William M. Snow

    2005-05-01

    The goal of this work, which is a collaborative effort between Indiana University, NIST, and Hamilton College, is to extend the technique of polarized neutron scattering into new domains by the development and application of polarized 3He-based neutron spin filters. After the IPNS experiment which measured Zeeman sp[litting in surface scattered neutrons using a polarized 3He cell as a polarization analyzer transporterd by car from Bloomington to Chicago, the Indiana work focused on technical developments to improve the 3He polarization of the Indiana compression system. The compression system was rebuilt with a new valve system which allows gas trapped in the dead volume of the compressors at the end of the piston stroke to be exhausted and conducted back to the optical pumping cell where it can be repolarized. We also incorporated a new intermediate storage volume made at NIST from 1720 glass which will reduce polarization losses between the compressors. Furthermore, we improved the stability of the 1083 nm laser by cooling the LMA rod. We achieved 60% 3he polarization in the optical pumping cell and 87% preservation of the polarization during compression. In parallel we built a magnetically-shielded transport solenoid for use on neutron scattering instruments such as POSY which achieves a fractional field uniformity of better than 10-3 per cm. The field was mapped using an automated 3D field mapping system for in-situ measurement of magnetic field gradients Diluted magnetic semiconductors offer many exciting opportunities for investigation of spintronic effects in solids and are certain to be one of the most active areas of condensed matter physics over then next several years. These materials can act as efficient spin injectors for devices that make use of spin-dependent transport phenomena. We just (late July 2002) finished a neutron reflectivity experiment at NIST on a GaMnAs trilayer film. This material is a ferromagnetic semiconductor which is of interest

  8. Precision measurement of the nuclear polarization in laser-cooled, optically pumped 37K

    NASA Astrophysics Data System (ADS)

    Fenker, B.; Behr, J. A.; Melconian, D.; Anderson, R. M. A.; Anholm, M.; Ashery, D.; Behling, R. S.; Cohen, I.; Craiciu, I.; Donohue, J. M.; Farfan, C.; Friesen, D.; Gorelov, A.; McNeil, J.; Mehlman, M.; Norton, H.; Olchanski, K.; Smale, S.; Thériault, O.; Vantyghem, A. N.; Warner, C. L.

    2016-07-01

    We report a measurement of the nuclear polarization of laser-cooled, optically pumped 37K atoms which will allow us to precisely measure angular correlation parameters in the {β }+-decay of the same atoms. These results will be used to test the V ‑ A framework of the weak interaction at high precision. At the Triumf neutral atom trap (Trinat), a magneto-optical trap confines and cools neutral 37K atoms and optical pumping spin-polarizes them. We monitor the nuclear polarization of the same atoms that are decaying in situ by photoionizing a small fraction of the partially polarized atoms and then use the standard optical Bloch equations to model their population distribution. We obtain an average nuclear polarization of \\bar{P}=0.9913+/- 0.0009, which is significantly more precise than previous measurements with this technique. Since our current measurement of the β-asymmetry has 0.2 % statistical uncertainty, the polarization measurement reported here will not limit its overall uncertainty. This result also demonstrates the capability to measure the polarization to \\lt 0.1 % , allowing for a measurement of angular correlation parameters to this level of precision, which would be competitive in searches for new physics.

  9. Polar confinement modulates solvation behavior of methane molecules

    NASA Astrophysics Data System (ADS)

    Xu, Weixin; Mu, Yuguang

    2008-06-01

    Polar confinement induces an amorphous solidlike state of water characterized by an orientational correlation time longer than hundreds of picoseconds and significant structural disorder. Solvation behavior of methane molecules is dramatically modulated under polar confinement. Moreover our simulations indicate that the charges equivalent to those borne by atoms of amino acids could generate an electric field which is strong enough to stimulate the phase transition of water. In our results, polar confinement is found to be more capable of aggregating hydrophobic molecules. This study raises an interesting mechanism by which the cagelike structure of the Escherichia coli chaperonin GroEL and the cochaperonin GroES complex helps protein folding.

  10. Onset of Ferrielectricity and the Hidden Nature of Nanoscale Polarization

    SciTech Connect

    Nunez, Matias

    2008-01-01

    Using calculations from first principles and the concept of layer polarization, we have elucidated the nanoscale organization and local polarization in ferroelectric thin films between metallic contacts. The profile of the local polarization for different film thicknesses unveils a peculiar spatial pattern of atomic layers with uncompensated dipoles in what was originally thought to be a ferroelectric domain. This effectively ferrielectric behavior is induced by the dominant roles of the interfaces at such reduced dimensionality and can be interpreted using a simple classical model where the latter are explicitly taken into account.

  11. Atomic Energy Basics, Understanding the Atom Series.

    ERIC Educational Resources Information Center

    Atomic Energy Commission, Oak Ridge, TN. Div. of Technical Information.

    This booklet is part of the "Understanding the Atom Series," though it is a later edition and not included in the original set of 51 booklets. A basic survey of the principles of nuclear energy and most important applications are provided. These major topics are examined: matter has molecules and atoms, the atom has electrons, the nucleus,…

  12. Polarization at the SLC

    SciTech Connect

    Moffeit, K.C.

    1988-10-01

    The Stanford Linear collider was designed to accommodate polarized electron beams. Longitudinally polarized electrons colliding with unpolarized positrons at a center of mass energy near the Z/sup 0/ mass can be used as novel and sensitive probes of the electroweak process. A gallium arsenide based photon emission source will provide a beam of longitudinally polarized electrons of about 45 percent polarization. A system of bend magnets and a superconducting solenoid will be used to rotate the spins so that the polarization is preserved while the 1.21 GeV electrons are stored in the damping ring. Another set of bend magnets and two superconducting solenoids orient the spin vectors so that longitudinal polarization of the electrons is achieved at the collision point with the unpolarized positrons. A system to monitor the polarization based on Moller and Compton scattering will be used. Nearly all major components have been fabricated and tested. Subsystems of the source and polarimeters have been installed, and studies are in progress. The installation and commissioning of the entire system will take place during available machine shutdown periods as the commissioning of SLC progresses. 8 refs., 16 figs., 1 tab.

  13. Light scattering from dense cold atomic media

    NASA Astrophysics Data System (ADS)

    Zhu, Bihui; Cooper, John; Ye, Jun; Rey, Ana Maria

    2016-08-01

    We theoretically study the propagation of light through a cold atomic medium, where the effects of motion, laser intensity, atomic density, and polarization can all modify the properties of the scattered light. We present two different microscopic models: the "coherent dipole model" and the "random-walk model", both suitable for modeling recent experimental work done in large atomic arrays in the low-light-intensity regime. We use them to compute relevant observables such as the linewidth, peak intensity, and line center of the emitted light. We further develop generalized models that explicitly take into account atomic motion. Those are relevant for hotter atoms and beyond the low-intensity regime. We show that atomic motion can lead to drastic dephasing and to a reduction of collective effects, together with a distortion of the line shape. Our results are applicable to model a full gamut of quantum systems that rely on atom-light interactions, including atomic clocks, quantum simulators, and nanophotonic systems.

  14. Modeling polarization reversal in optically pumped rubidium vapors

    NASA Astrophysics Data System (ADS)

    Dreiling, J. M.; Norrgard, E.; Gay, T. J.

    2010-03-01

    Rubidium atoms can be polarized by optical pumping with a resonant circularly polarized laser beam. Using Faraday rotation polarimetry [1], we have observed a flip in the sign of the Rb electron polarization when the wavelength of the pump laser is varied over the D1 absorption spectrum. This could occur if F < (I + J) states with MF = F are predominantly populated at specific pump frequencies resulting in different spin polarizations. We have used a simple rate equation model to estimate the final electron polarization under the assumption that we are able to pump only one F transition at a time. The results of these calculations will be presented. [4pt] [1] H. Batelaan, A.S. Green, B.A. Hitt, and T.J. Gay, Phys. Rev. Lett. 82, 4216 (1999).

  15. Polarized Photocathode R&D for Future Linear Collliders

    SciTech Connect

    Zhou, F; Brachmann, A.; Maruyama, T.; Sheppard, J.C.; /SLAC

    2009-01-23

    It is a challenge to generate full charge electrons from the electron sources without compromising polarization for the proposed ILC and CLIC. It is essential to advance polarized photocathodes to meet the requirements. SLAC has worldwide unique dedicated test facilities, Cathode Test System and dc-Gun Test Laboratory, to fully characterize polarized photocathodes. Recent systematic measurements on a strained-well InAlGaAs/AlGaAs cathode at the facilities show that 87% polarization and 0.3% QE are achieved. The QE can be increased to {approx}1.0% with atomic hydrogen cleaning. The surface charge limit at a very low current intensity and the clear dependence of the polarization on the surface charge limit are observed for the first time. On-going programs to develop photocathodes for the ILC and CLIC are briefly introduced.

  16. Intense, Narrow Atomic-Clock Resonances

    NASA Astrophysics Data System (ADS)

    Jau, Y.-Y.; Post, A. B.; Kuzma, N. N.; Braun, A. M.; Romalis, M. V.; Happer, W.

    2004-03-01

    We present experimental and theoretical results showing that magnetic resonance transitions from the “end” sublevels of maximum or minimum spin in alkali-metal vapors are a promising alternative to the conventional 0-0 transition for small-size gas-cell atomic clocks. For these “end resonances,” collisional spin-exchange broadening, which often dominates the linewidth of the 0-0 resonance, decreases with increasing spin polarization and vanishes for 100% polarization. The end resonances also have much stronger signals than the 0-0 resonance, and are readily detectable in cells with high buffer-gas pressure.

  17. North Polar Dunes

    NASA Technical Reports Server (NTRS)

    2006-01-01

    23 January 2006 This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) image shows dark sand dunes in the north polar region of Mars. Surrounding much of the north polar ice cap are fields of sand dunes. In this case, the strongest winds responsible for the dunes blew off the polar cap (not seen here), from the north-northwest (upper left).

    Location near: 76.5oN, 63.7oW Image width: 3 km (1.9 mi) Illumination from: lower left Season: Northern Summer

  18. GUIDE FOR POLARIZED NEUTRONS

    DOEpatents

    Sailor, V.L.; Aichroth, R.W.

    1962-12-01

    The plane of polarization of a beam of polarized neutrons is changed by this invention, and the plane can be flipped back and forth quicitly in two directions in a trouble-free manner. The invention comprises a guide having a plurality of oppositely directed magnets forming a gap for the neutron beam and the gaps are spaced longitudinally in a spiral along the beam at small stepped angles. When it is desired to flip the plane of polarization the magnets are suitably rotated to change the direction of the spiral of the gaps. (AEC)

  19. Coherent Control of Collective Atomic Spins

    NASA Astrophysics Data System (ADS)

    Trail, Collin M.

    2011-12-01

    In this thesis I explore the use of collective spin angular momentum as a platform for quantum information processing. In the limit of a large number of atoms, the collective variables of atomic systems have a natural connection to the bosonic algebra of light (known as the Holstein-Primakoff or HP approximation) where components of the collective spin angular momentum effectively act as quadratures, making them natural systems for coupling to light. I have sought to improve previous schemes for the spin squeezing of atomic ensembles, such as the proposal of Takeuchi et. al. based on coherent quantum feedback [39]. In this scheme a beam of linearly polarized light passes through the atomic ensemble (prepared in a coherent state), coupling to the atoms through a state-dependent index of refraction (the Faraday effect). The light is then passed through a wave-plate and reflected back through the atoms for a second pass. This double-pass scheme leads to an effective nonlinearity as the atomic fluctuations are mapped onto the light on the first pass and then back on to the atoms in the second pass. The light acts as a bus coupling each atom to each of the others. This nonlinear interaction forms a shearing of the atomic coherent state that results in squeezing. The light is entangled to the atoms through these interactions, and remains entangled as it escapes the system. This leads to decoherence of the atoms as the light is lost to the environment, reducing the amount of spin squeezing achieved. The first step towards improving the double-pass scheme was to add a quantum eraser step in which the light is disentangled from the squeezed atoms. By first measuring one quadrature of the light, and then performing a measurement-dependent rotation on the atomic ensemble, it is possible to decouple the atoms and light so that the loss of the light does not reduce the atomic squeezing. This results in an improvement of the rate of atomic spin squeezing. A complete model

  20. Polar Environmental Monitoring

    NASA Technical Reports Server (NTRS)

    Nagler, R. G.; Schulteis, A. C.

    1979-01-01

    The present and projected benefits of the polar regions were reviewed and then translated into information needs in order to support the array of polar activities anticipated. These needs included measurement sensitivities for polar environmental data (ice/snow, atmosphere, and ocean data for integrated support) and the processing and delivery requirements which determine the effectiveness of environmental services. An assessment was made of how well electromagnetic signals can be converted into polar environmental information. The array of sensor developments in process or proposed were also evaluated as to the spectral diversity, aperture sizes, and swathing capabilities available to provide these measurements from spacecraft, aircraft, or in situ platforms. Global coverage and local coverage densification options were studied in terms of alternative spacecraft trajectories and aircraft flight paths.

  1. Mercury's South Polar Region

    NASA Video Gallery

    This animation shows 89 wide-angle camera (WAC) images of Mercury’s south polar region acquired by the Mercury Dual Imaging System (MDIS) over one complete Mercury solar day (176 Earth days). Thi...

  2. Interferometric polarization control

    SciTech Connect

    Chuss, David T.; Wollack, Edward J.; Moseley, S. Harvey; Novak, Giles

    2006-07-20

    We develop the Jones and Mueller matrices for structures that allow control of the path length difference between two linear orthogonal polarizations and consider the effect of placing multiple devices in series. Specifically, we find that full polarization modulation (measurement of Stokes Q, U, and V) can be achieved by placing two such modulators in series if the relative angles of the beam-splitting grids with respect to the analyzer orientation are appropriately chosen. Such a device has several potential advantages over a spinning wave plate modulator for measuring astronomical polarization in the far infrared through millimeter: (i) The use of small, linear motions eliminates the need for cryogenic rotational bearings; (ii) the phase flexibility allows measurement of circular as well as linear polarization; and (iii) this architecture allows for both multiwavelength and broadband modulation. We also present initial laboratory results.

  3. Polarization contrast vision

    NASA Astrophysics Data System (ADS)

    Pugh, Edward N.

    1990-05-01

    An attempt is made to establish the possibility that the geometry of certain classes of vertebrate photoreceptors results in a birefringence that allows the animals to utilize the state of polarization of light striking their retinas as a meaningful stimulus parameter. Simulate the photoreceptors as dielectric waveguides using a simple physical model, and augment this theoretical work with empirical measurements of the light guiding properties of photoreceptors in isolated pieces of retina from a green sunfish (Lepomis cyanellus). With a classical conditioning paradigm, this fish's sensitivity to light is modulated by the orientation of the plane of polarization of linearly polarized light. This functional dependence was predicted by a hypothetical antagonistic mechanism between twin cones of two orientations in the animal's retinal mosaic. Further study is planned for the nature of the stimulus to which the fish is sensitive by creating a camera that will generate images based purely upon the contrast between orthogonal polarizations at each point in space.

  4. EDITORIAL: Polarization Optics

    NASA Astrophysics Data System (ADS)

    Turunen, Jari; Friesem, Asher A.; Friberg, Ari T.

    2004-03-01

    This special issue on Polarization Optics contains one review article and 23 research papers, many of which are based on presentations at the International Commission for Optics Topical Meeting on Polarization Optics, held in Polvijärvi, Finland, between 30 June and 3 July 2003. While this issue should not in any sense be considered as a `proceedings' of this meeting, the possibility of submitting papers to it was widely advertised during the meeting, which was attended by a large fraction of prominent scientists in the field of polarization optics. Thus the quality of papers in this special issue is high. In announcing both the meeting and this special issue, we emphasized that the concept of `polarization optics' should be understood in a wide sense. In fact, all contributions dealing with the vectorial nature of light were welcome. As a result, the papers included here cover a wide range of different aspects of linear and nonlinear polarization optics. Both theoretical and experimental features are discussed. We are pleased to see that the conference and this special issue both reflect the wide diversity of important and novel polarization phenomena in optics. The papers in this special issue, and other recently published works, demonstrate that even though polarization is a fundamental property of electromagnetic fields, interest in it is rapidly increasing. The fundamental relations between partial coherence and partial polarization are currently under vigorous research in electromagnetic coherence theory. In diffractive optics it has been found that the exploitation of the vectorial nature of light can be of great benefit. Fabrication of sophisticated, spatially variable polarization-control elements is becoming possible with the aid of nanolithography. Polarization singularities and the interplay of bulk properties and topology in nanoscale systems have created much enthusiasm. In nonlinear optics, the second harmonic waves generated on reflection and

  5. Observation of polar vortices in oxide superlattices

    NASA Astrophysics Data System (ADS)

    Yadav, A. K.; Nelson, C. T.; Hsu, S. L.; Hong, Z.; Clarkson, J. D.; Schlepüetz, C. M.; Damodaran, A. R.; Shafer, P.; Arenholz, E.; Dedon, L. R.; Chen, D.; Vishwanath, A.; Minor, A. M.; Chen, L. Q.; Scott, J. F.; Martin, L. W.; Ramesh, R.

    2016-02-01

    The complex interplay of spin, charge, orbital and lattice degrees of freedom provides a plethora of exotic phases and physical phenomena. In recent years, complex spin topologies have emerged as a consequence of the electronic band structure and the interplay between spin and spin-orbit coupling in materials. Here we produce complex topologies of electrical polarization—namely, nanometre-scale vortex-antivortex (that is, clockwise-anticlockwise) arrays that are reminiscent of rotational spin topologies—by making use of the competition between charge, orbital and lattice degrees of freedom in superlattices of alternating lead titanate and strontium titanate layers. Atomic-scale mapping of the polar atomic displacements by scanning transmission electron microscopy reveals the presence of long-range ordered vortex-antivortex arrays that exhibit nearly continuous polarization rotation. Phase-field modelling confirms that the vortex array is the low-energy state for a range of superlattice periods. Within this range, the large gradient energy from the vortex structure is counterbalanced by the corresponding large reduction in overall electrostatic energy (which would otherwise arise from polar discontinuities at the lead titanate/strontium titanate interfaces) and the elastic energy associated with epitaxial constraints and domain formation. These observations have implications for the creation of new states of matter (such as dipolar skyrmions, hedgehog states) and associated phenomena in ferroic materials, such as electrically controllable chirality.

  6. Polarization and Hyperfine Transitions of Metastable ^129Xe in Discharge Cells

    NASA Astrophysics Data System (ADS)

    Xia, Tian; Morgan, Steven; Jau, Yuan-Yu; Happer, William

    2010-03-01

    The polarization and relaxation rates of metastable ^129Xe atoms are measured with magnetic resonance spectroscopy, at both microwave frequencies, where δF = 1 transitions are induced between the sublevels, and at radiofrequencies, corresponding to δF = 0 transitions. The nuclear spin polarization of the resonant velocity group is measured to be 22±2%. However, the relaxation rate of spin polarization is much larger than the velocity changing rate, the narrow line pumping laser produces spin polarization only for atoms with resonant velocity. The relaxation of metastable xenon atoms is dominated by depolarizing collisions with ground state atoms, with lesser contributions from metastability exchange collisions. We also measure the pressure broadening coefficient of the relaxation rate by varying the temperature of the cryogenic part of the cell.

  7. Active polarization descattering.

    PubMed

    Treibitz, Tali; Schechner, Yoav Y

    2009-03-01

    Vision in scattering media is important but challenging. Images suffer from poor visibility due to backscattering and attenuation. Most prior methods for scene recovery use active illumination scanners (structured and gated), which can be slow and cumbersome, while natural illumination is inapplicable to dark environments. The current paper addresses the need for a non-scanning recovery method, that uses active scene irradiance. We study the formation of images under widefield artificial illumination. Based on the formation model, the paper presents an approach for recovering the object signal. It also yields rough information about the 3D scene structure. The approach can work with compact, simple hardware, having active widefield, polychromatic polarized illumination. The camera is fitted with a polarization analyzer. Two frames of the scene are taken, with different states of the analyzer or polarizer. A recovery algorithm follows the acquisition. It allows both the backscatter and the object reflection to be partially polarized. It thus unifies and generalizes prior polarization-based methods, which had assumed exclusive polarization of either of these components. The approach is limited to an effective range, due to image noise and illumination falloff. Thus, the limits and noise sensitivity are analyzed. We demonstrate the approach in underwater field experiments. PMID:19147870

  8. Fusion of a polarized projectile with a polarized target

    SciTech Connect

    Christley, J.A.; Johnson, R.C.; Thompson, I.J.

    1995-07-15

    The fusion cross sections for a polarized target with both unpolarized and polarized projectiles are studied. Expressions for the observables are given for the case when both nuclei are polarized. Calculations for fusion of an aligned {sup 165}Ho target with {sup 16}O and polarized {sup 7}Li beams are presented.

  9. Polarization effects in silver delafossite systems

    NASA Astrophysics Data System (ADS)

    Panapitiya, Gihan; Lewis, James P.

    Delafossites are a promising class of materials which has applications in catalysis and optoelectronic devices. Even though much work has been carried out on the cuprate family of delafossites, little is known about the structural and electronic properties of it's silver counterpart. In this work, we present a computational study for two delafossite oxides of the form AgB1 - x FexO2 (For B = Al,Ga). A large number of structures are studied by varying the Fe alloying percentage(x) from 0 to 5 and by choosing the impurity sites randomly. We find that the local structural changes occurring at the vicinity of Fe atoms in these two systems have opposite trends with regard to the O-O distance. The reason for this difference in the trends is identified as the polarization effects on the inter-atomic distances caused by the displacements in O atoms resulting from the incorporation of Fe in sites, previously occupied by either Al or Ga. We believe that these effects are mediated by the differences in the atomic radii of Fe, Al and Ga. Higher alloying levels coupled with nearest neighbor Fe atoms can intensify these distortions in the structure creating deformations in the O-Ag-O bonds, which are directly related to the formation of the conduction band edge in these systems.

  10. Rectilinear lattices of polarization vortices with various spatial polarization distributions.

    PubMed

    Fu, Shiyao; Zhang, Shikun; Wang, Tonglu; Gao, Chunqing

    2016-08-01

    In this paper, we propose a type of rectilinear lattices of polarization vortices, each spot in which has mutually independent, and controllable spatial polarization distributions. The lattices are generated by two holograms under special design. In the experiment, the holograms are encoded on two spatial light modulators, and the results fit very well with theory. Our scheme makes it possible to generate multiple polarization vortices with various polarization distributions simultaneously, for instance, radially and azimuthally polarized beams, and can be used in the domains as polarization-based data transmission system, optical manufacture, polarization detection and so on. PMID:27505812

  11. Continuum treatment of electronic polarization effect.

    PubMed

    Tan, Yu-Hong; Luo, Ray

    2007-03-01

    A continuum treatment of electronic polarization has been explored for in molecular mechanics simulations in implicit solvents. The dielectric constant for molecule interior is the only parameter in the continuum polarizable model. A value of 4 is found to yield optimal agreement with high-level ab initio quantum mechanical calculations for the tested molecular systems. Interestingly, its performance is not sensitive to the definition of molecular volume, in which the continuum electronic polarization is defined. In this model, quantum mechanical electrostatic field in different dielectric environments from vacuum, low-dielectric organic solvent, and water can be used simultaneously in atomic charge fitting to achieve consistent treatment of electrostatic interactions. The tests show that a single set of atomic charges can be used consistently in different dielectric environments and different molecular conformations, and the atomic charges transfer well from training monomers to tested dimers. The preliminary study gives us the hope of developing a continuum polarizable force field for more consistent simulations of proteins and nucleic acids in implicit solvents. PMID:17362100

  12. Continuum treatment of electronic polarization effect

    NASA Astrophysics Data System (ADS)

    Tan, Yu-Hong; Luo, Ray

    2007-03-01

    A continuum treatment of electronic polarization has been explored for in molecular mechanics simulations in implicit solvents. The dielectric constant for molecule interior is the only parameter in the continuum polarizable model. A value of 4 is found to yield optimal agreement with high-level ab initio quantum mechanical calculations for the tested molecular systems. Interestingly, its performance is not sensitive to the definition of molecular volume, in which the continuum electronic polarization is defined. In this model, quantum mechanical electrostatic field in different dielectric environments from vacuum, low-dielectric organic solvent, and water can be used simultaneously in atomic charge fitting to achieve consistent treatment of electrostatic interactions. The tests show that a single set of atomic charges can be used consistently in different dielectric environments and different molecular conformations, and the atomic charges transfer well from training monomers to tested dimers. The preliminary study gives us the hope of developing a continuum polarizable force field for more consistent simulations of proteins and nucleic acids in implicit solvents.

  13. ATOMIC BEAM STUDIES IN THE RHIC H-JET POLARIMETER.

    SciTech Connect

    MAKDISI,Y.; ZELENSKI,A.; GRAHAM,D.; KOKHANOVSKI,S.; MAHLER,G.; NASS,A.; RITTER,J.; ZUBETS,V.; ET AL.

    2005-01-28

    The results of atomic beam production studies are presented. Improved cooling of the atoms before jet formation in the dissociator cold nozzle apparently reduces the atomic beam velocity spread and improves beam focusing conditions. A carefully designed sextupole separating (and focusing) magnet system takes advantage of the high brightness source. As a result a record beam intensity of a 12.4 {center_dot} 10{sup 16} atoms/s was obtained within 10 mm acceptance at the collision point. The results of the polarization dilution factor measurements (by the hydrogen molecules at the collision point) are also presented.

  14. Ultracold-Atom Accelerometers

    NASA Technical Reports Server (NTRS)

    Noever, David A.

    1995-01-01

    Proposed class of accelerometers and related motion sensors based on use of ultracold atoms as inertial components of motion transducers. Ultracold atoms supplant spring-and-mass components of older accelerometers. As used here, "ultracold atoms" means atoms with kinetic energies equivalent to temperatures equal to or less than 20 mK. Acclerometers essentially frictionless. Primary advantage high sensitivity.

  15. Diffusive transfer of polarized 3He gas through depolarizing magnetic gradients

    NASA Astrophysics Data System (ADS)

    Maxwell, J. D.; Epstein, C. S.; Milner, R. G.

    2015-03-01

    Transfer of polarized 3He gas across spatially varying magnetic fields will facilitate a new source of polarized 3He ions for particle accelerators. In this context, depolarization of atoms as they pass through regions of significant transverse field gradients is a major concern. To understand these depolarization effects, we have built a system consisting of a Helmholtz coil pair and a solenoid, both with central magnetic fields of order 30 gauss. The atoms are polarized via metastability exchange optical pumping in the Helmholtz coil and are in diffusive contact via a glass tube with a second test cell in the solenoid. We have carried out measurements of the spin relaxation during transfer of polarization in 3He at 1 torr by diffusion. We explore the use of measurements of the loss of polarization taken in one cell to infer the polarization in the other cell.

  16. Polarized nuclear target based on parahydrogen induced polarization

    SciTech Connect

    D. Budker, M.P. Ledbetter, S. Appelt, L.S. Bouchard, B. Wojtsekhowski

    2012-12-01

    We discuss a novel concept of a polarized nuclear target for accelerator fixed-target scattering experiments, which is based on parahydrogen induced polarization (PHIP). One may be able to reach a 33% free-proton polarization in the ethane molecule. The potential advantages of such a target include operation at zero magnetic field, fast ({approx}100 HZ) polarization oscillation (akin to polarization reversal), and operation with large intensity of an electron beam.

  17. Polarized nuclear target based on parahydrogen induced polarization

    NASA Astrophysics Data System (ADS)

    Budker, D.; Ledbetter, M. P.; Appelt, S.; Bouchard, L. S.; Wojtsekhowski, B.

    2012-12-01

    We discuss a novel concept of a polarized nuclear target for accelerator fixed-target scattering experiments, which is based on parahydrogen induced polarization (PHIP). One may be able to reach a 33% free-proton polarization in the ethane molecule. The potential advantages of such a target include operation at zero magnetic field, fast (˜100 Hz) polarization oscillation (akin to polarization reversal), and operation with large intensity of an electron beam.

  18. Polar low dynamics

    SciTech Connect

    Montgomery, M.T.; Farrell, B.F. )

    1992-12-15

    Polar lows are intense subsynoptic-scale cyclones that form over high-latitude oceans in association with deep cumulus convection and strong ambient baroclinicity. Recent observations indicate that polar lows are generally initiated by a nonaxisymmetric interaction between a surface disturbance and an upper-level mobile trough. Extant theories of polar low formation preclude study of such a process since they either constrain their models to be axisymmetric, or do not explicitly account for his transient interaction. In this work the physics of interacting upper- and lower-level potential vorticity structures is studied as an initial-value problem using a three-dimensional nonlinear geostrophic momentum model that incorporates moist processes and includes strong baroclinic dynamics. Model results illustrate the rapid formation of an intense small-scale cyclone whose structure is consistent with observations of mature polar lows. A conceptual model of polar low development is proposed. In the first stage of development, called induced self-development, a mobile upper trough initiates a rapid low-level spinup due to the enhanced omega response in a conditionally neutral baroclinic atmosphere. A secondary development follows, called diabatic destabilization, that is associated with the production of low-level potential vorticity by diabatic processes. Diabatic destabilization represents a simple mechanism for maintaining the intensity of polar lows until they reach land. In exceptional instances of negligible upper-level forcing, the latter may also describe the gradual intensification of small-scale cyclones in regions of sustained neutrality and surface baroclinicity. Ideas regarding polar low equilibration and prospects for a unified theory of arctic and midlatitude cyclones are discussed. 75 refs., 4 figs., 1 tab.

  19. Sub-kilohertz laser linewidth narrowing using polarization spectroscopy.

    PubMed

    Torrance, Joshua S; Sparkes, Ben M; Turner, Lincoln D; Scholten, Robert E

    2016-05-30

    We identify several beneficial characteristics of polarization spectroscopy as an absolute atomic reference for frequency stabilization of lasers, and demonstrate sub-kilohertz laser spectral linewidth narrowing using polarization spectroscopy with high-bandwidth feedback. Polarization spectroscopy provides a highly dispersive velocity-selective absolute atomic reference based on frequency-dependent birefringence in an optically pumped atomic gas. The pumping process leads to dominance of the primary closed transition, suppressing closely-spaced subsidiary resonances which reduce the effective capture range for conventional atomic references. The locking signal is based on subtraction of two orthogonal polarization signals, reducing the effect of laser intensity noise to the shot noise limit. We measure noise-limited servo bandwidth comparable to that of a high-finesse optical cavity without the frequency limit or complexity imposed by optical modulation normally associated with high bandwidth laser frequency stabilization. We demonstrate narrowing to 600±100 Hz laser linewidth using the beatnote between two similarly locked external cavity diode lasers. PMID:27410068

  20. Collisional Properties of a Polarized Fermi Gas with Resonant Interactions

    SciTech Connect

    Bruun, G. M.; Recati, A.; Stringari, S.; Pethick, C. J.; Smith, H.

    2008-06-20

    Highly polarized mixtures of atomic Fermi gases constitute a novel Fermi liquid. We demonstrate how information on thermodynamic properties may be used to calculate quasiparticle scattering amplitudes even when the interaction is resonant and apply the results to evaluate the damping of the spin dipole mode. We estimate that under current experimental conditions the mode would be intermediate between the hydrodynamic and collisionless limits.

  1. A laser-driven source of polarized hydrogen and deuterium

    SciTech Connect

    Young, L.; Holt, R.J.; Gilman, R.A.; Kowalczyk, R.; Coulter, K.

    1989-01-01

    A novel laser-driven polarized source of hydrogen and deuterium which operates on the principle of spin-exchange optical pumping is being developed. This source is designed to operate as an internal target in an electron storage ring for fundamental studies of spin-dependent structure of nuclei. It has the potential to exceed the flux from existing conventional sources (3 /times/ 10/sup 16//s) by an order of magnitude. Currently, the source delivers hydrogen at a flux of 8 /times/ 10/sup 16/ atoms/s with an atomic polarization of 24% and deuterium at 6 /times/ 10/sup 16/ atoms/s with a polarization of 29%. Technical obstacles which have been overcome, with varying degrees of success are complete Doppler-coverage in the optical-pumping stage without the use of a buffer gas, wall-induced depolarization and radiation-trapping. Future improvements should allow achievement of the design goals of 4 /times/ 10/sup 17/ atoms/s with a polarization of 50%. 8 refs., 2 figs.

  2. Design and Development of a Microscopic Model for Polarization

    ERIC Educational Resources Information Center

    Petridou, E.; Psillos, D.; Hatzikraniotis, E.; Viiri, J.

    2009-01-01

    As research shows that the knowledge and use of models and modelling by teachers is limited, particularly for predicting phenomena, we developed and applied a sequence of three representations of a simulated model focusing on polarization and specifically showing the behaviour of an atom, and forces exerted on a dipole and an insulator, when a…

  3. Polarized Continuum Radiation from Stellar Atmospheres

    NASA Astrophysics Data System (ADS)

    Harrington, J. Patrick

    2015-10-01

    Continuum scattering by free electrons can be significant in early type stars, while in late type stars Rayleigh scattering by hydrogen atoms or molecules may be important. Computer programs used to construct models of stellar atmospheres generally treat the scattering of the continuum radiation as isotropic and unpolarized, but this scattering has a dipole angular dependence and will produce polarization. We review an accurate method for evaluating the polarization and limb darkening of the radiation from model stellar atmospheres. We use this method to obtain results for: (i) Late type stars, based on the MARCS code models (Gustafsson et al. 2008), and (ii) Early type stars, based on the NLTE code TLUSTY (Lanz and Hubeny 2003). These results are tabulated at http://www.astro.umd.edu/~jph/Stellar_Polarization.html. While the net polarization vanishes for an unresolved spherical star, this symmetry is broken by rapid rotation or by the masking of part of the star by a binary companion or during the transit of an exoplanet. We give some numerical results for these last cases.

  4. Sequential Polarity-Reversing Circuit

    NASA Technical Reports Server (NTRS)

    Labaw, Clayton C.

    1994-01-01

    Proposed circuit reverses polarity of electric power supplied to bidirectional dc motor, reversible electro-mechanical actuator, or other device operating in direction depending on polarity. Circuit reverses polarity each time power turned on, without need for additional polarity-reversing or direction signals and circuitry to process them.

  5. Cylindrically polarized nondiffracting optical pulses

    NASA Astrophysics Data System (ADS)

    Ornigotti, Marco; Conti, Claudio; Szameit, Alexander

    2016-07-01

    We extend the concept of radially and azimuthally polarized optical beams to the polychromatic domain by introducing cylindrically polarized nondiffracting optical pulses. In particular, we discuss in detail the case of cylindrically polarized X-waves, both in the paraxial and nonparaxial regime. The explicit expressions for the electric and magnetic fields of cylindrically polarized X-waves are also reported.

  6. Surface structures of polar and non-polar metal oxides

    NASA Astrophysics Data System (ADS)

    Chamberlin, Sara E.

    Metal oxides have long been a challenge to surface science since many traditional surface techniques are often affected by their insulating nature. In particular, high current electron beams can cause charging effects in addition to potentially desorbing surface species and damaging the surface. The development of a low current, low energy electron diffraction (LEED) system has allowed us to investigate metal oxide surfaces while significantly limiting the above mentioned complications. This low current LEED system has been used to perform a structural LEED-IV study of the reconstructed TiO2(011)-(2x1) surface. This surface is known to experience significant oxygen desorption when exposed to high current electron beams. The low current LEED system was crucial to maintain confidence in the structure found, which generally agreed with recently published models, but did not confirm one key feature. The oxygen atoms at the surface were not found to be asymmetrically bonded, which has been thought to be the cause of this surface's enhanced photocatalytic activity. We have also used the low current LEED system to investigate the polar oxide surfaces of ZnO(000 1¯) and MgO(111)-(✓3x✓3)R30°. For Zn0(000 1¯) LEED-IV structural study was combined with Density Functional Theory (DFT) calculations to investigate the impact of hydrogen on the surface. Our results support a disordered, fractional coverage of hydrogen terminating the surface. MgO(111)-(✓3x✓3)R30° has proven to be a challenging reconstructed surface. Both LEED-IV and surface x-ray diffraction (SXRD) find that previously proposed models for the surface are not a good fit to the data, so other models have been explored. The SXRD data in particular suggest that the reconstruction is more than one atomic layer deep.

  7. Neutral atom traps.

    SciTech Connect

    Pack, Michael Vern

    2008-12-01

    This report describes progress in designing a neutral atom trap capable of trapping sub millikelvin atom in a magnetic trap and shuttling the atoms across the atom chip from a collection area to an optical cavity. The numerical simulation and atom chip design are discussed. Also, discussed are preliminary calculations of quantum noise sources in Kerr nonlinear optics measurements based on electromagnetically induced transparency. These types of measurements may be important for quantum nondemolition measurements at the few photon limit.

  8. Josephson π state induced by valley polarization

    NASA Astrophysics Data System (ADS)

    Wang, Jun; Yang, Y. H.; Chan, K. S.

    2014-02-01

    We theoretically explore possible π-state Josephson junctions made from graphene-like two-dimensional materials (G) with the honeycomb lattice structure. It is shown that the valley polarization in the G sheet could lead to a 0-π state transition of the Josephson junction because of the valley-singlet Cooper pairs acquiring a nonzero momentum. When the valley-mixing scattering exists in the interfaces of the junction due to lattice mismatch, an odd-frequency valley-triplet supercurrent flows in the system even though the G sheet is fully valley polarized, and the supercurrent is characterized by a rapid atomic-scale oscillation with a periodicity of three lattice constants.

  9. Applications of Elliptically Polarized, Few-Cycle Attosecond Pulses

    NASA Astrophysics Data System (ADS)

    Starace, Anthony F.

    2016-05-01

    Use of elliptically-polarized light opens the possibility of investigating effects that are not accessible with linearly-polarized pulses. This talk presents two new physical effects that are predicted for ionization of the helium atom by few-cycle, elliptically polarized attosecond pulses. For double ionization of He by an intense elliptically polarized attosecond pulse, we predict a nonlinear dichroic effect (i.e., the difference of the two-electron angular distributions in the polarization plane for opposite helicities of the ionizing pulse) that is sensitive to the carrier-envelope phase, ellipticity, peak intensity I, and temporal duration of the pulse. For single ionization of He by two oppositely circularly polarized, time-delayed attosecond pulses we predict that the photoelectron momentum distributions in the polarization plane have helical vortex structures that are exquisitely sensitive to the time-delay between the pulses, their relative phase, and their handedness. Both of these effects manifest the ability to control the angular distributions of the ionized electrons by means of the attosecond pulse parameters. Our predictions are obtained numerically by solving the six-dimensional two-electron time-dependent Schrödinger equation for the case of elliptically polarized attosecond pulses. They are interpreted analytically by means of perturbation theory analyses of the two ionization processes. This work is supported in part by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Award No. DE-FG03-96ER14646.

  10. Polarization twist in perovskite ferrielectrics

    PubMed Central

    Kitanaka, Yuuki; Hirano, Kiyotaka; Ogino, Motohiro; Noguchi, Yuji; Miyayama, Masaru; Moriyoshi, Chikako; Kuroiwa, Yoshihiro

    2016-01-01

    Because the functions of polar materials are governed primarily by their polarization response to external stimuli, the majority of studies have focused on controlling polar lattice distortions. In some perovskite oxides, polar distortions coexist with nonpolar tilts and rotations of oxygen octahedra. The interplay between nonpolar and polar instabilities appears to play a crucial role, raising the question of how to design materials by exploiting their coupling. Here, we introduce the concept of ‘polarization twist’, which offers enhanced control over piezoelectric responses in polar materials. Our experimental and theoretical studies provide direct evidence that a ferrielectric perovskite exhibits a large piezoelectric response because of extended polar distortion, accompanied by nonpolar octahedral rotations, as if twisted polarization relaxes under electric fields. The concept underlying the polarization twist opens new possibilities for developing alternative materials in bulk and thin-film forms. PMID:27586824

  11. Polarization twist in perovskite ferrielectrics.

    PubMed

    Kitanaka, Yuuki; Hirano, Kiyotaka; Ogino, Motohiro; Noguchi, Yuji; Miyayama, Masaru; Moriyoshi, Chikako; Kuroiwa, Yoshihiro

    2016-01-01

    Because the functions of polar materials are governed primarily by their polarization response to external stimuli, the majority of studies have focused on controlling polar lattice distortions. In some perovskite oxides, polar distortions coexist with nonpolar tilts and rotations of oxygen octahedra. The interplay between nonpolar and polar instabilities appears to play a crucial role, raising the question of how to design materials by exploiting their coupling. Here, we introduce the concept of 'polarization twist', which offers enhanced control over piezoelectric responses in polar materials. Our experimental and theoretical studies provide direct evidence that a ferrielectric perovskite exhibits a large piezoelectric response because of extended polar distortion, accompanied by nonpolar octahedral rotations, as if twisted polarization relaxes under electric fields. The concept underlying the polarization twist opens new possibilities for developing alternative materials in bulk and thin-film forms. PMID:27586824

  12. Polar low monitoring

    NASA Astrophysics Data System (ADS)

    Bobylev, Leonid; Zabolotskikh, Elizaveta; Mitnik, Leonid

    2010-05-01

    Polar lows are intense mesoscale atmospheric low pressure weather systems, developing poleward of the main baroclinic zone and associated with high surface wind speeds. Small size and short lifetime, sparse in-situ observations in the regions of their development complicate polar low study. Our knowledge of polar lows and mesocyclones has come almost entirely during the period of satellite remote sensing since, by virtue of their small horizontal scale, it was rarely possible to analyse these lows on conventional weather charts using only the data from the synoptic observing network. However, the effects of intense polar lows have been felt by coastal communities and seafarers since the earliest times. These weather systems are thought to be responsible for the loss of many small vessels over the centuries, although the nature of the storms was not understood and their arrival could not be predicted. The actuality of the polar low research is stipulated by their high destructive power: they are a threat to such businesses as oil and gas exploration, fisheries and shipping. They could worsen because of global warming: a shrinking of sea ice around the North Pole, which thawed to its record minimum in the summer of 2007, is likely to give rise to more powerful storms that form only over open water and can cause hurricane-strength winds. Therefore, study of polar lows, their timely detection, tracking and forecasting represents a challenge for today meteorology. Satellite passive microwave data, starting from Special Sensor Microwave Imager (SSM/I) onboard Defense Meteorological Satellite Program (DMSP) satellite, remain invaluable source of regularly available remotely sensed data to study polar lows. The sounding in this spectral range has several advantages in comparison with observations in visible and infrared ranges and Synthetic Aperture Radar (SAR) data: independence on day time and clouds, regularity and high temporal resolution in Polar Regions. Satellite

  13. Studies on Beam Formation in an Atomic Beam Source

    SciTech Connect

    Nass, A.; Steffens, E.; Stancari, M.

    2009-08-04

    Atomic beam sources (ABS) are widely used workhorses producing polarized atomic beams for polarized gas targets and polarized ion sources. Although they have been used for decades the understanding of the beam formation processes is crude. Models were used more or less successfully to describe the measured intensity and beam parameters. ABS's are also foreseen for future experiments, such as PAX [1]. An increase of intensity at a high polarization would be beneficial. A direct simulation Monte-Carlo method (DSMC)[2] was used to describe the beam formation of a hydrogen or deuterium beam in an ABS. For the first time a simulation of a supersonic gas expansion on a molecular level for this application was performed. Beam profile and Time-of-Flight measurements confirmed the simulation results. Furthermore a new method of beam formation was tested, the Carrier Jet method [3], based on an expanded beam surrounded by an over-expanded carrier jet.

  14. The Hanle and Zeeman Polarization Signals of the Solar Ca II 8542 Å Line

    NASA Astrophysics Data System (ADS)

    Štěpán, Jiří; Trujillo Bueno, Javier

    2016-07-01

    We highlight the main results of a three-dimensional (3D) multilevel radiative transfer investigation about the solar disk-center polarization of the Ca ii 8542 Å line. First, through the use of a 3D model of the solar atmosphere, we investigate the linear polarization that occurs due to the atomic level polarization produced by the absorption and scattering of anisotropic radiation, taking into account the symmetry-breaking effects caused by its thermal, dynamic, and magnetic structure. Second, we study the contribution of the Zeeman effect to the linear and circular polarization. Finally, we show examples of the Stokes profiles produced by the joint action of the atomic level polarization and the Hanle and Zeeman effects. We find that the Zeeman effect tends to dominate the linear polarization signals only in the localized patches of opposite magnetic polarity, where the magnetic field is relatively strong and slightly inclined; outside such very localized patches, the linear polarization is often dominated by the contribution of atomic level polarization. We demonstrate that a correct modeling of this last contribution requires taking into account the symmetry-breaking effects caused by the thermal, dynamic, and magnetic structure of the solar atmosphere, and that in the 3D model used the Hanle effect in forward-scattering geometry (disk-center observation) mainly reduces the polarization corresponding to the zero-field case. We emphasize that, in general, a reliable modeling of the linear polarization in the Ca ii 8542 Å line requires taking into account the joint action of atomic level polarization and the Hanle and Zeeman effects.

  15. X-ray line polarization spectroscopy of Li-like satellite line spectra

    SciTech Connect

    Sherrill, Manolo Edgar; Abdallah, Joseph; Zhang, Honglin; Hakel, Peter; Mancini, Roberto C

    2008-01-01

    We apply the magnetic-sublevel atomic kinetics model POLAR to the calculation of polarization properties of satellite lines in Li-like Si driven by subpicosecond-duration laser pulses. We identify spectral lines whose polarization can serve as a marker of plasma anisotropy due to anisotropy in the electron distribution function. We also discuss the utility and limitations of ur current theoretical approach and point out possible future improvements and directions.

  16. Polarization of Starlight

    NASA Astrophysics Data System (ADS)

    Whittet, D. C. B.

    The polarization of starlight is universally attributed to directional extinction arising when dust grains along the line of sight are aligned in the presence of a magnetic field. This phenomenon provides a powerful tool for studying the optical properties of the dust (size, shape, refractive index) and for charting the galactic magnetic field. Current observational constraints at all wavelengths are consistent with a picture in which only the larger grains in the size range responsible for extinction are efficient polarizers. Small grains are much less well aligned and/or more isotropic in shape than large grains. The polarizing grains include silicates, but it is not clear whether they contain appreciable quantities of carbon. The degree of alignment is highly sensitive to ambient physical conditions as well as to particle size. The polarization efficiency per unit extinction declines with increasing density within dark clouds, hindering attempts to map the intracloud magnetic field. However, spectropolarimetric studies of interstellar ice absorption features seen in deeply embedded YSOs indicate that mantled grains within dense molecular clouds can be surprisingly efficient polarizers, suggesting that a qualitatively different alignment mechanism is operating compared with diffuse regions of the ISM. This talk will present a brief overview of key observations and their interpretation, highlight areas of uncertainty, and suggest avenues of future research. The physics of grain alignment is reviewed elsewhere in this meeting (see paper by Roberge).

  17. POLARBEAR CMB Polarization Experiment

    NASA Astrophysics Data System (ADS)

    Nishino, H.; Ade, P.; Akiba, Y.; Anthony, A.; Arnold, K.; Barron, D.; Boettger, D.; Borrill, J.; Chapmann, S.; Chinone, Y.; Dobbs, M. A.; Errard, J.; Fabbian, G.; Feng, C.; Flanigan, D.; Fuller, G.; Ghribi, A.; Grainger, W.; Halverson, N.; Hasegawa, M.; Hattori, K.; Hazumi, M.; Holzapfel, W. L.; Howard, J.; Hyland, P.; Inoue, Y.; Jaffe, A.; Jaehnig, G.; Kaneko, Y.; Katayama, N.; Keating, B.; Kermish, Z.; Kimura, N.; Kisner, T.; Lee, A. T.; Le Jeune, M.; Linder, E.; Lungu, M.; Matsuda, F.; Matsumura, T.; Miller, N. J.; Morii, H.; Moyerman, S.; Myers, M. J.; O'Brient, R.; Okamura, T.; Paar, H.; Peloton, J.; Quealy, E.; Reichardt, C. L.; Richards, P. L.; Ross, C.; Shimizu, A.; Shimon, M.; Shimmin, C.; Sholl, M.; Siritanasak, P.; Spieler, H.; Stebor, N.; Steinbach, B.; Stompor, R.; Suzuki, A.; Suzuki, J.; Tanaka, K.; Tomaru, T.; Tucker, C.; Yadav, A.; Zahn, O.

    POLARBEAR is a ground-based experiment in the Atacama desert in hile, measuring the polarization of the Cosmic Microwave Background (CMB) radiation. One of the science goals of POLARBEAR is to detect the B-mode polarization pattern of the CMB produced by primordial gravitational waves from the epoch of inflation. The detection of the B-mode polarization provides strong evidence for inflationary cosmological models. POLARBEAR is expected to reach a sensitivity to the tensor-to-scalar ratio r = 0.025 at 95% confidence level, using the data from two years of observation. With a beam size of 3.5 arcminutes, POLARBEAR is also sensitive to B-mode polarization signals at small-angular scales produced by weak gravitational lensing of large-scale structure. POLARBEAR is expected to provide a constraint on the sum of neutrino masses because of their effect on the large-scale structure. POLARBEAR was deployed in late 2011 and started observing in early 2012 at 150 GHz with an array of 1,274 polarization sensitive antenna-coupled Transition Edge Sensor (TES) bolometers. The current status of the POLARBEAR experiment is reported.

  18. Polarized protons at RHIC

    SciTech Connect

    Makdisi, Y.

    1992-10-01

    The approval for construction of the Relativistic Heavy Ion Collider (RHIC) provides a potential opportunity to collide polarized proton beams at energies up to 500 GeV in the center of mass and high luminosities approaching 2 {times} 10{sup 32}/cm{sup 2}/sec. This capability is enhanced by the fact that the AGS has already accelerated polarized protons and relies on the newly completed Accumulator/Booster for providing the required polarized proton intensity and a system of spin rotators (Siberian snakes) to retain the polarization. The RHIC Spin Collaboration was formed and submitted a Letter of Intent to construct this polarized collider capability and utilize its physics opportunities. In this presentation, I will discuss the plans to upgrade the AGS, the proposed layout of the RHIC siberian snakes, and timetables. The physics focus is the measurement of the spin dependent parton distributions with such accessible probes including high p(t) jets, direct photons, and Drell Yan. The attainable sensitivities and the progress that has been reached in defining the detector requirements will be outlined.

  19. Polarized protons at RHIC

    SciTech Connect

    Makdisi, Y.

    1992-01-01

    The approval for construction of the Relativistic Heavy Ion Collider (RHIC) provides a potential opportunity to collide polarized proton beams at energies up to 500 GeV in the center of mass and high luminosities approaching 2 {times} 10{sup 32}/cm{sup 2}/sec. This capability is enhanced by the fact that the AGS has already accelerated polarized protons and relies on the newly completed Accumulator/Booster for providing the required polarized proton intensity and a system of spin rotators (Siberian snakes) to retain the polarization. The RHIC Spin Collaboration was formed and submitted a Letter of Intent to construct this polarized collider capability and utilize its physics opportunities. In this presentation, I will discuss the plans to upgrade the AGS, the proposed layout of the RHIC siberian snakes, and timetables. The physics focus is the measurement of the spin dependent parton distributions with such accessible probes including high p(t) jets, direct photons, and Drell Yan. The attainable sensitivities and the progress that has been reached in defining the detector requirements will be outlined.

  20. A Compact Polarization Imager

    NASA Technical Reports Server (NTRS)

    Thompson, Karl E.; Rust, David M.; Chen, Hua

    1995-01-01

    A new type of image detector has been designed to analyze the polarization of light simultaneously at all picture elements (pixels) in a scene. The Integrated Dual Imaging Detector (IDID) consists of a polarizing beamsplitter bonded to a custom-designed charge-coupled device with signal-analysis circuitry, all integrated on a silicon chip. The IDID should simplify the design and operation of imaging polarimeters and spectroscopic imagers used, for example, in atmospheric and solar research. Other applications include environmental monitoring and robot vision. Innovations in the IDID include two interleaved 512 x 1024 pixel imaging arrays (one for each polarization plane), large dynamic range (well depth of 10(exp 6) electrons per pixel), simultaneous readout and display of both images at 10(exp 6) pixels per second, and on-chip analog signal processing to produce polarization maps in real time. When used with a lithium niobate Fabry-Perot etalon or other color filter that can encode spectral information as polarization, the IDID can reveal tiny differences between simultaneous images at two wavelengths.

  1. Artificial polarization components

    NASA Astrophysics Data System (ADS)

    Cescato, L.; Gluch, Ekkehard; Stork, Wilhelm; Streibl, Norbert

    1990-07-01

    High frequency surface relief structures are optically anisotropic and show interesting polarisation properties 1 . These properties can be used to produce polarizations components such as wave plates polarizers. polarizing beamsplitters etc. Our experimental results show that even gratings with relatively low spatial frequency ( periods A ) exhibit a strong phase retardation and can be used as quarter-wave plates. k INTRODUC11ON The artificial birefringence exhibited by ultrahigh frequency gratings of dielectric materials can be used to produce various polarization components2 . Such components have applications in integrated optics as well as in free space optics. In order to produce the high spatial frequencies complex processes such as electron-beam lithography and reactive ion etching are needed. We show in this paper that sinusoidal holographic gratings in photoresist exhibit also a strong phase ret even at relatively long periods. L EXPERIMENTAL MEASUREMENTS To obtain the phase retardation of a lower frequency ( period A ) grating a simple setup as used by Enger and 2 can be applied. In our case however there are three measurements necessary to obtain the phase retardation because transmission of the two perpendicularly polarized beams is different from each other. I GRATING PRODUCTION grating 2 3 4 5 6 7 8 9 period (pmj 0. 74 0. 74 0. 61 0. 54 0. 46 0. 32 0. 54 0. 54 0. 54 ne (sec) 60

  2. Microwave electric field sensing with Rydberg atoms

    NASA Astrophysics Data System (ADS)

    Stack, Daniel T.; Kunz, Paul D.; Meyer, David H.; Solmeyer, Neal

    2016-05-01

    Atoms form the basis of precise measurement for many quantities (time, acceleration, rotation, magnetic field, etc.). Measurements of microwave frequency electric fields by traditional methods (i.e. engineered antennas) have limited sensitivity and can be difficult to calibrate properly. Highly-excited (Rydberg) neutral atoms have very large electric-dipole moments and many dipole allowed transitions in the range of 1 - 500 GHz. It is possible to sensitively probe the electric field in this range using the combination of two quantum interference phenomena: electromagnetically induced transparency and the Autler-Townes effect. This technique allows for very sensitive field amplitude, polarization, and sub-wavelength imaging measurements. These quantities can be extracted by measuring properties of a probe laser beam as it passes through a warm rubidium vapor cell. Thus far, Rydberg microwave electrometry has relied upon the absorption of the probe laser. We report on our use of polarization rotation, which corresponds to the real part of the susceptibility, for measuring the properties of microwave frequency electric fields. Our simulations show that when a magnetic field is present and directed along the optical propagation direction a polarization rotation signal exists and can be used for microwave electrometry. One central advantage in using the polarization rotation signal rather than the absorption signal is that common mode laser noise is naturally eliminated leading to a potentially dramatic increase in signal-to-noise ratio.

  3. Atomic Physics 15: Proceedings of the Fifteenth International Conference on Atomic Physics.

    NASA Astrophysics Data System (ADS)

    van Linden van den Heuvell, H. B.; Walraven, J. T. M.; Reynolds, M. W.

    1997-07-01

    The Table of Contents for the full book PDF is as follows: * Preface * Generation of a "Schrödinger cat" of radiation and observation of its decoherence * Synthesis of entangled states and quantum computing * Entangled states of atomic ions for quantum metrology and computation * Entanglement and indistinguishability: Coherence experiments with photon pairs and triplets * Atom optics as a testing ground for quantum chaos * Coherent ultra-bright XUV lasers and harmonics * Hollow atoms * Interdisciplinary experiments with polarized noble gases * The creation and study of Bose-Einstein condensation in a cold alkali vapor * oscopic quantum phenomena in trapped Bose-condensed gases * Doppler-free spectroscopy of trapped atomic hydrogen * QED and the ground state of helium * Towards coherent atomic samples using laser cooling * Bose-Einstein condensation of a weakly-interacting gas * Zeeman and his contemporaries: Dutch physics around 1900 * Zeeman's great discovery * The Zeeman effect: A tool for atom manipulation * The Zeeman effect a century later: New insights into classical physics * QED effects in few-electron high-Z systems * Lamb shift experiments on high-Z one- and two-electron systems * Fundamental constants of nature * Response of atoms in photonic lattices * Hydrogen-like systems and quantum electrodynamics * New experiments with atomic lattices bound by light * Bloch oscillations of atoms in an optical potential * Quantum decoherence and inertial sensing with atom interferometers * Quantum effects in He clusters * Atoms in super-intense radiation fields * Wave packet dynamics of excited atomic electrons in intense laser fields * Nonlinear laser-electron scattering * Comparing the antiproton and proton and progress toward cold antihydrogen * Author Index

  4. Polarized beams at RHIC

    SciTech Connect

    Roser, T.

    1995-11-01

    The Relativistic Heavy Ion Collider (RHIC) at Brookhaven allows for the unique possibility of colliding two 250 GeV polarized proton beams at luminosities of up to 2 {times} 10{sup 32} cm{sup {minus}2} s{sup {minus}1}. A partial Siberian Snake in the AGS has recently been successfully tested and full Siberian Snakes, spin rotators, and polarimeters for RHIC are being developed to make the acceleration of polarized beams to 250 GeV possible. High energy polarized beam collisions will open up the unique physics opportunities of studying spin effects in hard processes, which will allow the study of the spin structure of the proton and also the verification of the many well documented expectations of spin effects in perturbative QCD and parity violation in W and Z production.

  5. A lunar polar expedition

    NASA Technical Reports Server (NTRS)

    Dowling, Richard; Staehle, Robert L.; Svitek, Tomas

    1992-01-01

    Advanced exploration and development in harsh environments require mastery of basic human survival skill. Expeditions into the lethal climates of Earth's polar regions offer useful lessons for tommorrow's lunar pioneers. In Arctic and Antarctic exploration, 'wintering over' was a crucial milestone. The ability to establish a supply base and survive months of polar cold and darkness made extensive travel and exploration possible. Because of the possibility of near-constant solar illumination, the lunar polar regions, unlike Earth's may offer the most hospitable site for habitation. The World Space Foundation is examining a scenario for establishing a five-person expeditionary team on the lunar north pole for one year. This paper is a status report on a point design addressing site selection, transportation, power, and life support requirements.

  6. South Polar Layers

    NASA Technical Reports Server (NTRS)

    2003-01-01

    MGS MOC Release No. MOC2-516, 17 October 2003

    This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) image shows eroded, stair-stepped layers in the south polar region of Mars. These layers have been considered, for the past three decades, to consist of a mixture of dust and ice. The Mars Polar Lander (MPL) mission was designed to test this hypothesis. However, sadly, MPL was lost during descent in December 1999. This exposure of south polar layered material is located near 86.3oS, 187.7oW. The image covers an area 3 km (1.9 mi) wide and is illuminated by sunlight from the upper left.

  7. Polarized Light from Jupiter

    NASA Technical Reports Server (NTRS)

    2001-01-01

    These images taken through the wide angle camera near closest approach in the deep near-infrared methane band, combined with filters which sense electromagnetic radiation of orthogonal polarization, show that the light from the poles is polarized. That is, the poles appear bright in one image, and dark in the other. Polarized light is most readily scattered by aerosols. These images indicate that the aerosol particles at Jupiter's poles are small and likely consist of aggregates of even smaller particles, whereas the particles at the equator and covering the Great Red Spot are larger. Images like these will allow scientists to ascertain the distribution, size and shape of aerosols, and consequently, the distribution of heat, in Jupiter's atmosphere.

  8. South Polar Scarps

    NASA Technical Reports Server (NTRS)

    2003-01-01

    MGS MOC Release No. MOC2-438, 31 July 2003

    The terrain of the south polar residual ice cap, made up mostly of frozen carbon dioxide, has come to be known by many as 'swiss cheese terrain,' because many areas of the cap resemble slices of swiss cheese. However, not all of the south polar cap looks like a tasty lunch food. This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) image shows a series of curving scarps formed by erosion and sublimation of carbon dioxide from the south polar cap. This area is located near 86.3oS, 51.2oW. The image is illuminated by sunlight from the upper left; the area is about 1.5 km (0.9 mi) wide.

  9. Diurnal polar motion

    NASA Technical Reports Server (NTRS)

    Mcclure, P.

    1973-01-01

    An analytical theory is developed to describe diurnal polar motion in the earth which arises as a forced response due to lunisolar torques and tidal deformation. Doodson's expansion of the tide generating potential is used to represent the lunisolar torques. Both the magnitudes and the rates of change of perturbations in the earth's inertia tensor are included in the dynamical equations for the polar motion so as to account for rotational and tidal deformation. It is found that in a deformable earth with Love's number k = 0.29, the angular momentum vector departs by as much as 20 cm from the rotation axis rather than remaining within 1 or 2 cm as it would in a rigid earth. This 20 cm separation is significant in the interpretation of submeter polar motion observations because it necessitates an additional coordinate transformation in order to remove what would otherwise be a 20 cm error source in the conversion between inertial and terrestrial reference systems.

  10. Spring polar ozone behavior

    NASA Technical Reports Server (NTRS)

    Aikin, Arthur C.

    1992-01-01

    Understanding of the springtime behavior of polar stratospheric ozone as of mid 1990 is summarized. Heterogeneous reactions on polar stratospheric clouds as hypothesis for ozone loss are considered and a simplified description of the behavior of Antarctic ozone in winter and spring is given. Evidence that the situation is more complicated than described by the theory is produced. Many unresolved scientific issues remain and some of the most important problems are identified. Ozone changes each spring since 1979 have clearly established for the first time that man made chlorine compounds influence stratospheric ozone. Long before important advances in satellite and in situ investigations, it was Dobson's decision to place a total ozone measuring spectrometer at Halley Bay in Antarctica during the International Geophysical Year and subsequent continuous monitoring which led to the discovery that ozone was being destroyed each spring by chlorine processed by polar stratospheric clouds.

  11. Optical Production of Ultracold Polar Molecules

    SciTech Connect

    Sage, Jeremy M.; Sainis, Sunil; DeMille, David; Bergeman, Thomas

    2005-05-27

    We demonstrate the production of ultracold polar RbCs molecules in their vibronic ground state, via photoassociation of laser-cooled atoms followed by a laser-stimulated state transfer process. The resulting sample of X{sup 1}{sigma}{sup +}(v=0) molecules has a translational temperature of {approx}100 {mu}K and a narrow distribution of rotational states. With the method described here it should be possible to produce samples even colder in all degrees of freedom, as well as other bialkali species.

  12. Photonic, Electronic and Atomic Collisions

    NASA Astrophysics Data System (ADS)

    Fainstein, Pablo D.; Lima, Marco Aurelio P.; Miraglia, Jorge E.; Montenegro, Eduardo C.; Rivarola, Roberto D.

    2006-11-01

    Plenary. Electron collisions - past, present and future / J. W. McConkey. Collisions of slow highly charged ions with surfaces / J. Burgdörfer ... [et al.]. Atomic collisions studied with "reaction-microscopes" / R. Moshammer ... [et al.]. Rydberg atoms: a microscale laboratory for studying electron-molecule tnteractions / F. B. Dunning -- Collisions involvintg photons. Quantum control of photochemical reaction dynamics and molecular functions / M. Yamaki ... [et al.]. Manipulating and viewing Rydberg wavepackets / R. R. Jones. Angle-resolved photoelectrons as a probe of strong-field interactions / M. Vrakking. Ultracold Rydberg atoms in a structured environment / I. C. H. Liu and J. M. Rost. Synchrotron-radiation-based recoil ion momentum spectroscopy of laser cooled and trapped cesium atoms / L. H. Coutinho. Reconstruction of attosecond pulse trains / Y. Mairesse ... [et al.]. Selective excitation of metastable atomic states by Femto- and attosecond laser pulses / A. D. Kondorskiy. Accurate calculations of triple differential cross sections for double photoionization of the hygrogen molecule / W. Vanroose ... [et al.]. Double and triple photoionization of Li and Be / J. Colgan, M. S. Pindzola and F. Robicheaux. Few/many body dynamics in strong laser fields / J. Zanghellini and T. Brabec. Rescattering-induced effects in electron-atom scattering in the presence of a circularly polarized laser field / A. V. Flegel ... [et al.]. Multidimensional photoelectron spectroscopy / P. Lablanquie ... [et al.]. Few photon and strongly driven transitions in the XUV and beyond / P. Lambropoulos, L. A. A. Nikolopoulos and S. I. Themelis. Ionization dynamics of atomic clusters in intense laser pulses / U. Saalmann and J. M. Rost. On the second order autocorrelation of an XUV attosecond pulse train / E. P. Benis ... [et al.]. Evidence for rescattering in molecular dissociation / I. D. Williams ... [et al.]. Photoionizing ions using synchrotron radiation / R. Phaneuf. Photo double

  13. POLARIZED NEUTRONS IN RHIC

    SciTech Connect

    COURANT,E.D.

    1998-04-27

    There does not appear to be any obvious way to accelerate neutrons, polarized or otherwise, to high energies by themselves. To investigate the behavior of polarized neutrons the authors therefore have to obtain them by accelerating them as components of heavier nuclei, and then sorting out the contribution of the neutrons in the analysis of the reactions produced by the heavy ion beams. The best neutron carriers for this purpose are probably {sup 3}He nuclei and deuterons. A polarized deuteron is primarily a combination of a proton and a neutron with their spins pointing in the same direction; in the {sup 3}He nucleus the spins of the two protons are opposite and the net spin (and magnetic moment) is almost the same as that of a free neutron. Polarized ions other than protons may be accelerated, stored and collided in a ring such as RHIC provided the techniques proposed for polarized proton operation can be adapted (or replaced by other strategies) for these ions. To accelerate polarized particles in a ring, one must make provisions for overcoming the depolarizing resonances that occur at certain energies. These resonances arise when the spin tune (ratio of spin precession frequency to orbit frequency) resonates with a component present in the horizontal field. The horizontal field oscillates with the vertical motion of the particles (due to vertical focusing); its frequency spectrum is dominated by the vertical oscillation frequency and its modulation by the periodic structure of the accelerator ring. In addition, the magnet imperfections that distort the closed orbit vertically contain all integral Fourier harmonics of the orbit frequency.

  14. Generation of entangled squeezed states: their entanglement and quantum polarization

    NASA Astrophysics Data System (ADS)

    Karimi, A.; Tavassoly, M. K.

    2015-11-01

    In this paper, based on the well-known one-mode and two-mode squeezed states, we introduce the two-mode and four-mode entangled squeezed states. Next, in order to generate the introduced entangled states, we present two theoretical schemes based on the resonant atom-field interaction. In the proposed schemes, a Λ -type three-level atom interacts with the two-mode and four-mode quantized field in the presence of two strong classical fields in which two-photon atomic transitions are allowed. In the continuation, we study entanglement dynamics of the generated entangled states (using the von Neumann entropy) as well as the quantum polarization (using the Stokes operators). It is demonstrated that entanglement and polarization can be achieved for the produced states by adjusting the evolved parameters.

  15. Microwave Frequency Polarizers

    NASA Technical Reports Server (NTRS)

    Ha, Vien The; Mirel, Paul; Kogut, Alan J.

    2013-01-01

    This article describes the fabrication and analysis of microwave frequency polarizing grids. The grids are designed to measure polarization from the cosmic microwave background. It is effective in the range of 500 to 1500 micron wavelength. It is cryogenic compatible and highly robust to high load impacts. Each grid is fabricated using an array of different assembly processes which vary in the types of tension mechanisms to the shape and size of the grids. We provide a comprehensive study on the analysis of the grids' wire heights, diameters, and spacing.

  16. South Polar Variety

    NASA Technical Reports Server (NTRS)

    2005-01-01

    28 July 2005 This Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) image shows a view of linear troughs and mesas formed in the frozen carbon dioxide of the martian south polar residual cap. This image, obtained in May 2005, is a reminder that not all of the south polar cap landscapes resemble 'swiss cheese.'

    Location near: 86.7oS, 24.8oW Image width: width: 3 km (1.9 mi) Illumination from: upper left Season: Southern Spring

  17. Ultracold polar KRb molecules

    NASA Astrophysics Data System (ADS)

    Neyenhuis, Brian; Chotia, Amodsen; Moses, Steven; Ye, Jun; Jin, Deborah

    2011-05-01

    Ultracold polar molecules in the quantum degenerate regime open the possibility of realizing quantum gases with long-range, and spatially anisotropic, interparticle interactions. Currently, we can create a gas of ultracold fermionic ground-state KRb molecules in with a peak density of 1012 cm-3 and a temperature just 1.4 times the Fermi temperature. We will report on efforts to further cool this gas of molecules. One possibility is to evaporatively cool a spin-polarized molecular Fermi gas confined in quasi-2D, where we would rely on dipole-dipole interactions for rethermalization. We acknowledge funding from NIST, NSF, and AFOSR-MURI.

  18. Polarization encoded color camera.

    PubMed

    Schonbrun, Ethan; Möller, Guðfríður; Di Caprio, Giuseppe

    2014-03-15

    Digital cameras would be colorblind if they did not have pixelated color filters integrated into their image sensors. Integration of conventional fixed filters, however, comes at the expense of an inability to modify the camera's spectral properties. Instead, we demonstrate a micropolarizer-based camera that can reconfigure its spectral response. Color is encoded into a linear polarization state by a chiral dispersive element and then read out in a single exposure. The polarization encoded color camera is capable of capturing three-color images at wavelengths spanning the visible to the near infrared. PMID:24690806

  19. Physics with Polarized Antiprotons

    SciTech Connect

    Lenisa, Paolo

    2008-04-30

    Polarized antiprotons will provide access to a wealth of double- (and single-) spin observables, thereby opening a window to physics uniquely accessible with the HESR at FAIR. This include a first direct measurement of the transversity distribution of the valence quarks in the proton and a first measurement of the moduli and phase of the time-like electric and magnetic form factors G{sub E,M} of the proton. Additional applications of a polarized antiproton beam can be forseen in hadron spectroscopy, and nucleon-antinucleon scattering.

  20. Femtosecond polarization pulse shaping.

    PubMed

    Brixner, T; Gerber, G

    2001-04-15

    We report computer-controlled femtosecond polarization pulse shaping where intensity, momentary frequency, and light polarization are varied as functions of time. For the first time to our knowledge, a pulse shaper is used to modulate the degree of ellipticity as well as the orientation of the elliptical principal axes within a single laser pulse by use of a 256-pixel two-layer liquid-crystal display inside a zero-dispersion compressor. Interferometric stability of the setup is not required. Complete pulse characterization is achieved by dual-channel spectral interferometry. This technology has a large range of applications, especially in the field of quantum control. PMID:18040384