Pressure-Induced Order in the Gapped Quantum Magnet DTN
NASA Astrophysics Data System (ADS)
Mannig, Alexandra; Moeller, Johannes; Zheludev, Andrey; Garlea, V. Ovidiu; Dela Cruz, Clarina; Guguchia, Zurab; Khasanov, Rustem; Morenzoni, Elvezio
We present muon-spin relaxation, neutron diffraction and magnetic susceptibility data under applied hydrostatic pressure on the organometallic S = 1 quantum magnet NiCl2 . 4 [ SC(NH2)2 ] . The material consists of weakly coupled antiferromagnetic chains and has a spin gap resulting from a large single-ion anisotropy. Our muon spin rotation experiments provide local field dependencies on temperature as well as pressure and allow for the mapping of a detailed phase diagram up to 22kbar. Thus, we demonstrate that the compound may be driven through two subsequent pressure-induced transitions into apparently distinct magnetically ordered phases. Neutron diffraction and susceptibility measurements support those results and show the potential of low-pressure transitions to be investigated by various techniques.
NASA Astrophysics Data System (ADS)
O'Neal, K. R.; Zhou, J.; Cherian, J. G.; Turnbull, M. M.; Landee, C. P.; Jena, P.; Liu, Z.; Musfeldt, J. L.
2016-03-01
We combined synchrotron-based infrared and Raman spectroscopies, diamond anvil cell techniques, and first principles calculations to unveil pressure-induced distortions in quasi-one-dimensional Cu(pyz)(NO3)2. The crossover at 0.7 GPa is local in nature whereas the transition at 5 GPa lowers symmetry from P m n a to P 2221 and is predicted to slightly increase magnetic dimensionality. Comparison with prior magnetoinfrared results reveals the striking role of out-of-plane bending of the pyrazine ligand, a finding that we discuss in terms of the possibility of using pressure to bias the magnetic quantum critical transition in this classic S =1 /2 antiferromagnet.
Pressure-induced magnetic instability in Pd-Ni alloys
NASA Astrophysics Data System (ADS)
Oomi, Gendo; Iwai, Sadanori; Ohashi, Masashi; Nakano, Tomohito
2012-12-01
The electrical resistivity ρ(T) of dilute Pd-Ni alloys has been measured at high pressure up to 3 GPa. It is found that the ρ(T) of the ferromagnetic Pd-Ni alloy shows an anomalous temperature dependence near the critical pressure Pc, where the ferromagnetism disappears. The results are analysed in the framework of quantum critical behaviour induced by pressure. The effect of magnetic field on the ρ(T) is also examined. Different behaviour of magnetoresistance against pressure was found depending on the alloy concentration and discussed in connection with an instability of ferromagnetism.
Quantum Oscillation Signatures of Pressure-induced Topological Phase Transition in BiTeI
Park, Joonbum; Jin, Kyung-Hwan; Jo, Y. J.; Choi, E. S.; Kang, W.; Kampert, E.; Rhyee, J.-S.; Jhi, Seung-Hoon; Kim, Jun Sung
2015-01-01
We report the pressure-induced topological quantum phase transition of BiTeI single crystals using Shubnikov-de Haas oscillations of bulk Fermi surfaces. The sizes of the inner and the outer FSs of the Rashba-split bands exhibit opposite pressure dependence up to P = 3.35 GPa, indicating pressure-tunable Rashba effect. Above a critical pressure P ~ 2 GPa, the Shubnikov-de Haas frequency for the inner Fermi surface increases unusually with pressure, and the Shubnikov-de Haas oscillations for the outer Fermi surface shows an abrupt phase shift. In comparison with band structure calculations, we find that these unusual behaviors originate from the Fermi surface shape change due to pressure-induced band inversion. These results clearly demonstrate that the topological quantum phase transition is intimately tied to the shape of bulk Fermi surfaces enclosing the time-reversal invariant momenta with band inversion. PMID:26522628
Ab initio study of pressure-induced magnetic transition in manganese pnictides
NASA Astrophysics Data System (ADS)
Prathiba, G.; Naanci, B. Anto; Rajagopalan, M.
2007-02-01
We report a density functional calculation on the NiAs-type Mn-based pnictides. The total energy as a function of volume is obtained by means of self-consistent tight-binding linear muffin-tin orbital method by performing spin and non-spin polarized calculation. From the present study, we predict a magnetic-phase transition from ferromagnetic (FM) to non-magnetic (NM) around 49 and 35.7 GPa for MnAs and MnSb, respectively. The pressure-induced transition is found to be a second-order transition. The band structure and density of states (DOS) are plotted for FM and NM states. Apart from this the ground-state properties like magnetic moment, lattice parameter and bulk modulus are calculated and are compared with the available results. Under large volume expansion these compounds exist in zinc-blende (ZB) structure, which shows half metallicity. The magnetic moment and equilibrium lattice constants for ZB structure are obtained as well as band structure and DOS are presented.
Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds
NASA Astrophysics Data System (ADS)
Chi, Songxue; Uwatoko, Yoshiya; Cao, Huibo; Hirata, Yasuyuki; Hashizume, Kazuki; Aoyama, Takuya; Ohgushi, Kenya
2016-07-01
The pressure effects on the antiferromagentic orders in iron-based ladder compounds CsFe2Se3 and BaFe2S3 have been studied using neutron diffraction. With identical crystal structure and similar magnetic structures, the two compounds exhibit highly contrasting magnetic behaviors under moderate external pressures. In CsFe2Se3 the ladders are brought much closer to each other by pressure, but the stripe-type magnetic order shows no observable change. In contrast, the stripe order in BaFe2S3 undergoes a quantum phase transition where an abrupt increase of Néel temperature by more than 50% occurs at about 1 GPa, accompanied by a jump in the ordered moment. With its spin structure unchanged, BaFe2S3 enters an enhanced magnetic phase that bears the characteristics of an orbital selective Mott phase, which is the true neighbor of superconductivity emerging at higher pressures.
Magnetic Precursor of the Pressure-Induced Superconductivity in Fe-Ladder Compounds.
Chi, Songxue; Uwatoko, Yoshiya; Cao, Huibo; Hirata, Yasuyuki; Hashizume, Kazuki; Aoyama, Takuya; Ohgushi, Kenya
2016-07-22
The pressure effects on the antiferromagentic orders in iron-based ladder compounds CsFe_{2}Se_{3} and BaFe_{2}S_{3} have been studied using neutron diffraction. With identical crystal structure and similar magnetic structures, the two compounds exhibit highly contrasting magnetic behaviors under moderate external pressures. In CsFe_{2}Se_{3} the ladders are brought much closer to each other by pressure, but the stripe-type magnetic order shows no observable change. In contrast, the stripe order in BaFe_{2}S_{3} undergoes a quantum phase transition where an abrupt increase of Néel temperature by more than 50% occurs at about 1 GPa, accompanied by a jump in the ordered moment. With its spin structure unchanged, BaFe_{2}S_{3} enters an enhanced magnetic phase that bears the characteristics of an orbital selective Mott phase, which is the true neighbor of superconductivity emerging at higher pressures. PMID:27494496
NASA Astrophysics Data System (ADS)
Gilder, S. A.; Egli, R.; Hochleitner, R.; Roud, S. C.; Volk, M. W. R.; Le Goff, M.; de Wit, M.
2012-04-01
Meteorites and diamonds encounter high pressures during their formation or subsequent evolution. These materials sometimes contain magnetic inclusions of pyrrhotite. Because magnetic properties are sensitive to strain, pyrrhotite can potentially record the shock or formation pressures of its host. Moreover, pyrrhotite undergoes a pressure-induced phase transition between 1.6 and 6.2 GPa, but the magnetic signature of this transition is poorly known. Here we report room temperature magnetic measurements on multi- and single domain pyrrhotite under non-hydrostatic pressure up to 4.5 GPa. We find that the ratio of magnetic coercivity and remanence follows a logarithmic law with respect to pressure, which can potentially be used as a geobarometer. Due to the greater thermal expansion of pyrrhotite with respect to diamond, pyrrhotite inclusions in diamond experience a confining pressure at the Earth's surface. Applying our experimentally derived magnetic geobarometer to pyrrhotite-bearing diamonds from Botswana and the Central African Republic suggests the pressures of the pyrrhotite inclusions in the diamonds range from 1.3 to 2.1 GPa. These overpressures constrain the mantle source pressures from 5.4 to 9.5 GPa, depending on which bulk modulus and thermal expansion coefficients of the two phases are used. We are now trying to develop magnetic barometers on other magnetic phases to apply to meteorites, ultimately to constrain the minimum pressure in which the meteorite formed and, hence, information regarding the planetesmal's size, and/or depth, in which the meteorite was derived.
NASA Astrophysics Data System (ADS)
Gilder, S. A.; Egli, R.; Hochleitner, R.; Roud, S. C.; Volk, M.; Le Goff, M.; de Wit, M.
2010-12-01
Meteorites and diamonds encounter high-pressures during their geologic histories. These materials commonly contain magnetic inclusions of pyrrhotite, and because magnetic properties are sensitive to strain, pyrrhotite can potentially record the shock or formation pressures of its host. Moreover, pyrrhotite undergoes a pressure-induced phase transition between 1.6 and 6.2 GPa, but the magnetic signature of this transition is poorly known. Here we report magnetic measurements performed at high-pressures on single and multi-domain pyrrhotite. A magnetic hysteresis model based on our observations suggests that multidomain pyrrhotite transforms into single domain-like material, and once in the single domain state, hysteresis loops become progressively squarer and then squatter with increasing pressure, until they ultimately collapse approaching the paramagnetic state at the transition. The ratio of the bulk magnetic coercive force to magnetic remanence for pure pyrrhotite is reversible with pressure and follows a logarithmic law as a function of pressure, which can be used as a magnetic barometer for natural systems.
NASA Astrophysics Data System (ADS)
Vignesh, G.; Nithiananthi, P.
2016-04-01
The influence of pressure along the growth axis on carrier localization in GaAs/Al0.3Ga0.7As Double Quantum Well (DQW) is studied under strongly coupled regime and isolated regimes of the well. The effective mass approximation combined with variation technique is adopted with the inclusion of mismatches in effective mass and dielectric constants of the well and barrier material. Effect of the barrier and well on carrier localization is investigated by observing the diamagnetic susceptibility (χdia) for various impurity locations (zi) and the critical limit of the barrier (Lb ≈ 50 Å) for tunneling has also been estimated. The effect of Γ-Χ crossover due to the application of pressure on the donor localization is picturized through diamagnetic susceptibility.
Pressure-induced phonon softenings and the structural and magnetic transitions in CrO2
NASA Astrophysics Data System (ADS)
Kim, Sooran; Kim, Kyoo; Kang, Chang-Jong; Min, B. I.
2012-03-01
To investigate the pressure-induced structural transitions of chromium dioxide (CrO2), phonon dispersions and total-energy band structures are calculated as a function of pressure. The observed structural transition has been theoretically reproduced at P≈10 GPa from the ground-state tetragonal CrO2 (t-CrO2) of the rutile type to orthorhombic CrO2 (o-CrO2) of the CaCl2 type. The half-metallic property is found to be preserved in o-CrO2. The softening of the Raman-active B1g phonon mode, which is responsible for this structural transition, is demonstrated. The second structural transition is found to occur for P⩾61.1 GPa from ferromagnetic (FM) o-CrO2 to nonmagnetic monoclinic CrO2 (m-CrO2) of the MoO2 type, which is related to the softening mode at q=R((1)/(2),0,(1)/(2)). The third structural transition has been identified at P=88.8 GPa from m-CrO2 to cubic CrO2 of the CaF2 type that is a FM insulator.
Pressure-induced electronic phase separation of magnetism and superconductivity in CrAs
Khasanov, Rustem; Guguchia, Zurab; Eremin, Ilya; Luetkens, Hubertus; Amato, Alex; Biswas, Pabitra K.; Ruegg, Christian; Susner, Michael A.; Sefat, Athena S.; Zhigadlo, Nikolai D.; Morenzoni, Elvezio
2015-09-08
We report that the recent discovery of pressure (p) induced superconductivity in the binary helimagnet CrAs has raised questions on how superconductivity emerges from the magnetic state and on the mechanism of the superconducting pairing. In the present work the suppression of magnetism and the occurrence of superconductivity in CrAs were studied by means of muon spin rotation. The magnetism remains bulk up to p ≃ 3.5 kbar while its volume fraction gradually decreases with increasing pressure until it vanishes at p ≃ 7 kbar. At 3.5 kbar superconductivity abruptly appears with its maximum T_{c} ≃ 1.2 K which decreases upon increasing the pressure. In the intermediate pressure region (3.5≲ p ≲ 7 kbar) the superconducting and the magnetic volume fractions are spatially phase separated and compete for phase volume. Our results indicate that the less conductive magnetic phase provides additional carriers (doping) to the superconducting parts of the CrAs sample thus leading to an increase of the transition temperature (T_{c}) and of the superfluid density (ρ_{s}). A scaling of ρ_{s} with T_{c}^{3.2} as well as the phase separation between magnetism and superconductivity point to a conventional mechanism of the Cooper-pairing in CrAs.
Pressure-induced electronic phase separation of magnetism and superconductivity in CrAs.
Khasanov, Rustem; Guguchia, Zurab; Eremin, Ilya; Luetkens, Hubertus; Amato, Alex; Biswas, Pabitra K; Rüegg, Christian; Susner, Michael A; Sefat, Athena S; Zhigadlo, Nikolai D; Morenzoni, Elvezio
2015-01-01
The recent discovery of pressure (p) induced superconductivity in the binary helimagnet CrAs has raised questions on how superconductivity emerges from the magnetic state and on the mechanism of the superconducting pairing. In the present work the suppression of magnetism and the occurrence of superconductivity in CrAs were studied by means of muon spin rotation. The magnetism remains bulk up to p ≃ 3.5 kbar while its volume fraction gradually decreases with increasing pressure until it vanishes at p ≃ 7 kbar. At 3.5 kbar superconductivity abruptly appears with its maximum Tc ≃ 1.2 K which decreases upon increasing the pressure. In the intermediate pressure region (3.5 < or ~ p < or ~ 7 kbar) the superconducting and the magnetic volume fractions are spatially phase separated and compete for phase volume. Our results indicate that the less conductive magnetic phase provides additional carriers (doping) to the superconducting parts of the CrAs sample thus leading to an increase of the transition temperature (Tc) and of the superfluid density (ρs). A scaling of ρs with Tc(3.2) as well as the phase separation between magnetism and superconductivity point to a conventional mechanism of the Cooper-pairing in CrAs. PMID:26346548
Pressure-induced electronic phase separation of magnetism and superconductivity in CrAs
Khasanov, Rustem; Guguchia, Zurab; Eremin, Ilya; Luetkens, Hubertus; Amato, Alex; Biswas, Pabitra K.; Rüegg, Christian; Susner, Michael A.; Sefat, Athena S.; Zhigadlo, Nikolai D.; Morenzoni, Elvezio
2015-01-01
The recent discovery of pressure (p) induced superconductivity in the binary helimagnet CrAs has raised questions on how superconductivity emerges from the magnetic state and on the mechanism of the superconducting pairing. In the present work the suppression of magnetism and the occurrence of superconductivity in CrAs were studied by means of muon spin rotation. The magnetism remains bulk up to p 3.5 kbar while its volume fraction gradually decreases with increasing pressure until it vanishes at p 7 kbar. At 3.5 kbar superconductivity abruptly appears with its maximum Tc 1.2 K which decreases upon increasing the pressure. In the intermediate pressure region (3.5 p 7 kbar) the superconducting and the magnetic volume fractions are spatially phase separated and compete for phase volume. Our results indicate that the less conductive magnetic phase provides additional carriers (doping) to the superconducting parts of the CrAs sample thus leading to an increase of the transition temperature (Tc) and of the superfluid density (ρs). A scaling of ρs with as well as the phase separation between magnetism and superconductivity point to a conventional mechanism of the Cooper-pairing in CrAs. PMID:26346548
Pressure-induced electronic phase separation of magnetism and superconductivity in CrAs
Khasanov, Rustem; Guguchia, Zurab; Eremin, Ilya; Luetkens, Hubertus; Amato, Alex; Biswas, Pabitra K.; Ruegg, Christian; Susner, Michael A.; Sefat, Athena S.; Zhigadlo, Nikolai D.; et al
2015-09-08
We report that the recent discovery of pressure (p) induced superconductivity in the binary helimagnet CrAs has raised questions on how superconductivity emerges from the magnetic state and on the mechanism of the superconducting pairing. In the present work the suppression of magnetism and the occurrence of superconductivity in CrAs were studied by means of muon spin rotation. The magnetism remains bulk up to p ≃ 3.5 kbar while its volume fraction gradually decreases with increasing pressure until it vanishes at p ≃ 7 kbar. At 3.5 kbar superconductivity abruptly appears with its maximum Tc ≃ 1.2 K which decreasesmore » upon increasing the pressure. In the intermediate pressure region (3.5≲ p ≲ 7 kbar) the superconducting and the magnetic volume fractions are spatially phase separated and compete for phase volume. Our results indicate that the less conductive magnetic phase provides additional carriers (doping) to the superconducting parts of the CrAs sample thus leading to an increase of the transition temperature (Tc) and of the superfluid density (ρs). A scaling of ρs with Tc3.2 as well as the phase separation between magnetism and superconductivity point to a conventional mechanism of the Cooper-pairing in CrAs.« less
Jung, Soon-Gil; Kang, Ji-Hoon; Park, Eunsung; Lee, Sangyun; Lin, Jiunn-Yuan; Chareev, Dmitriy A; Vasiliev, Alexander N; Park, Tuson
2015-01-01
We investigate the relation of the critical current density (Jc) and the remarkably increased superconducting transition temperature (Tc) for the FeSe single crystals under pressures up to 2.43 GPa, where the Tc is increased by ~8 K/GPa. The critical current density corresponding to the free flux flow is monotonically enhanced by pressure which is due to the increase in Tc, whereas the depinning critical current density at which the vortex starts to move is more influenced by the pressure-induced magnetic state compared to the increase of Tc. Unlike other high-Tc superconductors, FeSe is not magnetic, but superconducting at ambient pressure. Above a critical pressure where magnetic state is induced and coexists with superconductivity, the depinning Jc abruptly increases even though the increase of the zero-resistivity Tc is negligible, directly indicating that the flux pinning property compared to the Tc enhancement is a more crucial factor for an achievement of a large Jc. In addition, the sharp increase in Jc in the coexisting superconducting phase of FeSe demonstrates that vortices can be effectively trapped by the competing antiferromagnetic order, even though its antagonistic nature against superconductivity is well documented. These results provide new guidance toward technological applications of high-temperature superconductors. PMID:26548444
Jung, Soon-Gil; Kang, Ji-Hoon; Park, Eunsung; Lee, Sangyun; Lin, Jiunn-Yuan; Chareev, Dmitriy A.; Vasiliev, Alexander N.; Park, Tuson
2015-01-01
We investigate the relation of the critical current density (Jc) and the remarkably increased superconducting transition temperature (Tc) for the FeSe single crystals under pressures up to 2.43 GPa, where the Tc is increased by ~8 K/GPa. The critical current density corresponding to the free flux flow is monotonically enhanced by pressure which is due to the increase in Tc, whereas the depinning critical current density at which the vortex starts to move is more influenced by the pressure-induced magnetic state compared to the increase of Tc. Unlike other high-Tc superconductors, FeSe is not magnetic, but superconducting at ambient pressure. Above a critical pressure where magnetic state is induced and coexists with superconductivity, the depinning Jc abruptly increases even though the increase of the zero-resistivity Tc is negligible, directly indicating that the flux pinning property compared to the Tc enhancement is a more crucial factor for an achievement of a large Jc. In addition, the sharp increase in Jc in the coexisting superconducting phase of FeSe demonstrates that vortices can be effectively trapped by the competing antiferromagnetic order, even though its antagonistic nature against superconductivity is well documented. These results provide new guidance toward technological applications of high-temperature superconductors. PMID:26548444
Pressure-Induced Enhanced Magnetic Anisotropy in Mn(N(CN)2)2
Quintero, P. A.; Rajan, D.; Peprah, M. K.; Brinzari, T. V.; Fishman, Randy Scott; Talham, Daniel R.; Meisel, Mark W.
2015-01-01
Using DC and AC magnetometry, the pressure dependence of the magnetization of the threedimensional antiferromagnetic coordination polymer Mn(N(CN)2)2 was studied up to 12 kbar and down to 8 K. The magnetic transition temperature, Tc, increases dramatically with applied pressure (P), where a change from Tc(P = ambient) = 16:0 K to Tc(P = 12:1 kbar) = 23:5 K was observed. In addition, a marked difference in the magnetic behavior is observed above and below 7.1 kbar. Specifically, for P < 7:1 kbar, the differences between the field-cooled and zero-field-cooled (fc-zfc) magnetizations, the coercive field, and the remanent magnetization decrease with increasing pressure. However, for P > 7:1 kbar, the behavior is inverted. Additionally, for P > 8:6 kbar, minor hysteresis loops are observed. All of these effects are evidence of the increase of the superexchange interaction and the appearance of an enhanced exchange anisotropy with applied pressure.
Strong cooperative coupling of pressure-induced magnetic order and nematicity in FeSe.
Kothapalli, K; Böhmer, A E; Jayasekara, W T; Ueland, B G; Das, P; Sapkota, A; Taufour, V; Xiao, Y; Alp, E; Bud'ko, S L; Canfield, P C; Kreyssig, A; Goldman, A I
2016-01-01
A hallmark of the iron-based superconductors is the strong coupling between magnetic, structural and electronic degrees of freedom. However, a universal picture of the normal state properties of these compounds has been confounded by recent investigations of FeSe where the nematic (structural) and magnetic transitions appear to be decoupled. Here, using synchrotron-based high-energy x-ray diffraction and time-domain Mössbauer spectroscopy, we show that nematicity and magnetism in FeSe under applied pressure are indeed strongly coupled. Distinct structural and magnetic transitions are observed for pressures between 1.0 and 1.7 GPa and merge into a single first-order transition for pressures ≳1.7 GPa, reminiscent of what has been found for the evolution of these transitions in the prototypical system Ba(Fe1-xCox)2As2. Our results are consistent with a spin-driven mechanism for nematic order in FeSe and provide an important step towards a universal description of the normal state properties of the iron-based superconductors. PMID:27582003
Pressure induced magnetic and semiconductor–metal phase transitions in Cr2MoO6
NASA Astrophysics Data System (ADS)
San-Dong, Guo
2016-05-01
We investigate magnetic ordering and electronic structures of Cr2MoO6 under hydrostatic pressure. To overcome the band gap problem, the modified Becke and Johnson exchange potential is used to investigate the electronic structures of Cr2MoO6. The insulating nature at the experimental crystal structure is produced, with a band gap of 1.04 eV, and the magnetic moment of the Cr atom is 2.50 μ B, compared to an experimental value of about 2.47 μ B. The calculated results show that an antiferromagnetic inter-bilayer coupling–ferromagnetic intra-bilayer coupling to a ferromagnetic inter-bilayer coupling–antiferromagnetic intra-bilayer coupling phase transition is produced with the pressure increasing. The magnetic phase transition is simultaneously accompanied by a semiconductor–metal phase transition. The magnetic phase transition can be explained by the Mo–O hybridization strength, and ferromagnetic coupling between two Cr atoms can be understood by empty Mo-d bands perturbing the nearest O-p orbital. Project supported by the Fundamental Research Funds for the Central Universities, China (Grant No. 2015XKMS073).
Structural response in FeCl2 (iron chloride) to pressure-induced electro-magnetic transitions
Taylor, R D; Rozenberg, G Kh; Pasternak, M P; Gorodetsky, P; Xu, W M; Dubrovinsky, L S; Le Bihan, T L
2009-01-01
High pressure (HP) synchrotron x-ray diffraction studies were carried out in FeCl{sub 2} together with resistivity (R) studies, at various temperatures and pressures to 65 GPa using diamond anvil cells. This work follows a previous HP {sup 57}Fe Mossbauer study in which two pressure-induced (PI) electronic transitions were found interpreted as: (i) quenching of the orbital-term contribution to the hyperfine field concurring with a tilting of the magnetic moment by 55 degrees and (ii) collapse of the magnetism concurring with a sharp decrease of the isomer shift (IS). The R(P,T) studies affirm that the cause the collapse of the magnetism is a PI p-d correlation breakdown, leading to an insulator-metal transition at {approx}45 GPa and is not due to a spi-Ir,crossover (S=2 {yields} S=0). The structure response to the pressure evolution of the two electronic phase transitions starting at low pressures (LP), through an intermediate phase (IP) 30-57 GPa, and culminating in a high-pressure phase (HP), P >32 GPa, can clearly be quantified. The IP-HP phases coexist through the 32-57 GPa range in which the HP abundance increases monotonically at the expense of the IP phase. At the LP-IP interface no volume change is detected, yet the c-axis increases and the a-axis shrinks by 0.21 Angstroms and 0.13 Angstroms, respectively. The fit of the equation of state of the combined LP-IP phases yields a bulk modulus K{sub 0} = 35.3(1.8) GPa. The intralayer CI-CI distances increases, but no change is observed in Fe-CI bond-length nor are there substantial changes in the interlayer spacing. The pressure-induced electronic IP-HP transition leads to a first-order structural phase transition characterized by a decrease in Fe-CI bond length and an abrupt drop in V(P) by {approx}3.5% accompanying the correlation breakdown. In this transition no symmetry change is detected,and the XRD data could be satisfactorily fitted with the CdI{sub 2} structure. The bulk modulus of the HP phase is
Pressure-Induced Phase Transition in a Molecule-Based Magnet with Interpenetrating Sublattices
Fishman, Randy Scott; Shum, William W.; Miller, Joel S.
2010-01-01
The molecule-based magnet [Ru2(O2CMe)4]3[Cr(CN)6] contains two interpenetrating sublattices with each sublattice moment confined by anisotropy to a cubic diagonal. At ambient pressure, a field of about 850 Oe rotates the antiferromagnetically-coupled sublattice moments towards the field direction, producing a wasp-waisted magnetization curve. Up to 7 kbar, the sublattice moments increase with pressure due to the enhanced exchange coupling between the Cr and Ru2 spins on each sublattice. Above 7 kbar, the sublattice moment drops by about half and the the linear susceptibility of each sublattice along the cubic diagonal increases dramatically. The most likely explanation for this phase transition is that a high- to low-spin transition on each Ru2 complex reverses and lowers the net spin of each sublattice.
Pressure-induced magnetic transitions with change of the orbital configuration in dimerised systems
NASA Astrophysics Data System (ADS)
Korotin, Dmitry M.; Anisimov, Vladimir I.; Streltsov, Sergey V.
2016-05-01
We suggest a possible scenario for magnetic transition under pressure in dimerised systems where electrons are localised on molecular orbitals. The mechanism of transition is not related with competition between kinetic energy and on-site Coulomb repulsion as in Mott-Hubbard systems, or between crystal-field splitting and intra-atomic exchange as in classical atomic spin-state transitions. Instead, it is driven by the change of bonding-antibonding splitting on part of the molecular orbitals. In the magnetic systems with few half-filled molecular orbitals external pressure may result in increase of the bonding-antibonding splitting and localise all electrons on low-lying molecular orbitals suppressing net magnetic moment of the system. We give examples of the systems, where this or inverse transition may occur and by means of ab initio band structure calculations predict that it can be observed in α‑MoCl4 at pressure P ~ 11 GPa.
Pressure-induced magnetic transitions with change of the orbital configuration in dimerised systems
Korotin, Dmitry M.; Anisimov, Vladimir I.; Streltsov, Sergey V.
2016-01-01
We suggest a possible scenario for magnetic transition under pressure in dimerised systems where electrons are localised on molecular orbitals. The mechanism of transition is not related with competition between kinetic energy and on-site Coulomb repulsion as in Mott-Hubbard systems, or between crystal-field splitting and intra-atomic exchange as in classical atomic spin-state transitions. Instead, it is driven by the change of bonding-antibonding splitting on part of the molecular orbitals. In the magnetic systems with few half-filled molecular orbitals external pressure may result in increase of the bonding-antibonding splitting and localise all electrons on low-lying molecular orbitals suppressing net magnetic moment of the system. We give examples of the systems, where this or inverse transition may occur and by means of ab initio band structure calculations predict that it can be observed in α−MoCl4 at pressure P ~ 11 GPa. PMID:27189206
Pressure-induced magnetic transitions with change of the orbital configuration in dimerised systems.
Korotin, Dmitry M; Anisimov, Vladimir I; Streltsov, Sergey V
2016-01-01
We suggest a possible scenario for magnetic transition under pressure in dimerised systems where electrons are localised on molecular orbitals. The mechanism of transition is not related with competition between kinetic energy and on-site Coulomb repulsion as in Mott-Hubbard systems, or between crystal-field splitting and intra-atomic exchange as in classical atomic spin-state transitions. Instead, it is driven by the change of bonding-antibonding splitting on part of the molecular orbitals. In the magnetic systems with few half-filled molecular orbitals external pressure may result in increase of the bonding-antibonding splitting and localise all electrons on low-lying molecular orbitals suppressing net magnetic moment of the system. We give examples of the systems, where this or inverse transition may occur and by means of ab initio band structure calculations predict that it can be observed in α-MoCl4 at pressure P ~ 11 GPa. PMID:27189206
Gao, L.; Chen, B.; Wang, J.; Alp, E.E.; Zhao, J.; Lerche, M.; Sturhahn, W.; Scott, H.P.; Huang, F.; Ding, Y.; Sinogeikin, S.V.; Lundstrom, C.C.; Bass, J.D.; Li, J.; X-Ray Science Division; Univ. of Illinois; Carnegie Inst. of Washington; Indiana Univ.
2008-09-11
We have carried out nuclear resonant scattering measurements on {sup 57}Fe-enriched Fe{sub 3}C between 1 bar and 50 GPa at 300 K. Synchrotron Moessbauer spectra reveal a pressure-induced magnetic transition in Fe{sub 3}C between 4.3 and 6.5 GPa. On the basis of our nuclear resonant inelastic X-ray scattering spectra and existing equation-of-state data, we have derived the compressional wave velocity V{sub p} and shear wave velocity V{sub s} for the high-pressure nonmagnetic phase, which can be expressed as functions of density ({rho}): V{sub p} (km/s) = -3.99 + 1.29{rho}(g/cm{sup 3}) and V{sub s} (km/s) = 1.45 + 0.24{rho}(g/cm{sup 3}). The addition of carbon to iron-nickel alloy brings density, V{sub p} and V{sub s} closer to seismic observations, supporting carbon as a principal light element in the Earth's inner core.
NASA Astrophysics Data System (ADS)
Zou, T.; Cao, H. B.; Liu, G. Q.; Peng, J.; Gottschalk, M.; Zhu, M.; Zhao, Y.; Leão, J. B.; Tian, W.; Mao, Z. Q.; Ke, X.
2016-07-01
We report the hydrostatic pressure-induced electronic and magnetic phase transitions in a Mott insulator, a bilayer ruthenate C a3(Ru0.97Ti0.03 ) 2O7 , via electronic transport and single crystal neutron diffraction measurements. The system undergoes an insulator-metal transition at a very small hydrostatic pressure ≈0.04 GPa, followed by a magnetic phase transition around 0.3 GPa, suggesting that the low energy charge fluctuation and magnetic ordering couple to the pressure separately in this compound. The a b initio calculations show that the suppressed Ru O6 flattening induced by the pressure reduces the orbital polarization and gives rise to an insulator-metal transition preceding the magnetic phase transition.
Magnetically driven quantum heat engine
NASA Astrophysics Data System (ADS)
Munoz, Enrique; Pena, Francisco
2015-03-01
In analogy with classical thermodynamics, a quantum heat engine generates useful mechanical work from heat, by means of a reversible sequence of transformations (trajectories), where the ``working substance'' is of quantum mechanical nature. Several theoretical implementations for a quantum heat engine have been discussed in the literature, such as entangled states in a qubit, quantum mechanical versions of the Otto cycle, and photocells. In this work, we propose yet a different alternative by introducing the concept of a magnetically driven quantum heat engine. We studied the efficiency of such system, by considering as the ``working substance'' a single nonrelativistic particle trapped in a cylindrical potential well, as a model for a semiconductor quantum dot, in the presence of an external magnetic field. The trajectories are driven by a quasistatic modulation of the external magnetic-field intensity, while the system is in contact with macroscopic thermostats. The external magnetic field modulation allows to modify the effective geometric confinement, in analogy with a piston in a classical gas. E. Munoz acknowledges financial support from Fondecyt under Contract 1141146.
Simultaneous Pressure-Induced Magnetic and Valence Transitions in Type-I Clathrate Eu8Ga16Ge30
NASA Astrophysics Data System (ADS)
Onimaru, Takahiro; Tsutsui, Satoshi; Mizumaki, Masaichiro; Kawamura, Naomi; Ishimatsu, Naoki; Avila, Marcos A.; Yamamoto, Shuhei; Yamane, Haruki; Suekuni, Koichiro; Umeo, Kazunori; Kume, Tetsuji; Nakano, Satoshi; Takabatake, Toshiro
2014-01-01
We have performed X-ray magnetic circular dichroism (XMCD) and X-ray absorption spectroscopy (XAS) measurements at pressures up to 17 GPa for the clathrate Eu8Ga16Ge30 (Curie temperature TC = 36 K). The temperature dependence of the XMCD spectra agrees well with that of the DC magnetization at ambient pressure. The TC is gradually enhanced with increasing pressures up to 13.3 GPa, and the divalent state of the Eu ions with J = 7/2 remains stable, but at 17 GPa the XMCD intensity is strongly suppressed and a spectral weight corresponding to the trivalent state of Eu ions (with no magnetic moment) appears in the XAS spectrum. The concurrent change from the type-I clathrate structure to an amorphous phase has been observed by X-ray diffraction experiment. We conclude that the amorphization of this compound induces the mixed valence state, which collapses the ferromagnetism.
NASA Astrophysics Data System (ADS)
Rozenberg, G. Kh.; Pasternak, M. P.; Gorodetsky, P.; Xu, W. M.; Dubrovinsky, L. S.; Le Bihan, T.; Taylor, R. D.
2009-06-01
High-pressure (HP) synchrotron x-ray diffraction (XRD) studies were carried out in FeCl2 (TN≈24K) together with resistivity (R) studies at various temperatures and pressures to 65 GPa using diamond-anvil cells. This work follows a previous HP F57e Mössbauer study in which two pressure-induced (PI) electronic transitions were found interpreted as: (i) quenching of the orbital-term contribution to the hyperfine field concurring with a tilting of the magnetic moment by 55° , and (ii) collapse of the magnetism concurring with a sharp decrease in the isomer shift. The R(P,T) studies affirm that the cause of the collapse of the magnetism is a PI p-d correlation breakdown, leading to an insulator-metal transition at ˜45GPa and is not due to a spin crossover (S=2→S=0) . The structure response to the pressure evolution of the two electronic phase transitions starting at low pressures (LP), through an intermediate phase (IP) 30-57 GPa, and culminating in a high-pressure phase, P>32GPa , can clearly be quantified. The IP-HP phases coexist through the 32-57 GPa range in which the HP abundance increases monotonically at the expense of the IP phase. At the LP-IP interface no volume change is detected, yet the c axis increases and the a axis shrinks by 0.21 and 0.13Å , respectively. The fit of the equation of state of the combined LP-IP phases yields a bulk modulus K0=35.3(1.8)GPa . The intralayer Cl-Cl distances increase but no change is observed in Fe-Cl bond length nor are there substantial changes in the interlayer spacing. The pressure-induced electronic IP-HP transition leads to a first-order structural phase transition characterized by a decrease in Fe-Cl bond length and an abrupt drop in V(P) by ˜3.5% accompanying the correlation breakdown. In this transition no symmetry change is detected and the XRD data could be satisfactorily fitted with the CdI2 structure. The bulk modulus of the HP phase is practically the same as that of the LP-IP phases suggesting
Magnetically driven quantum heat engine.
Muñoz, Enrique; Peña, Francisco J
2014-05-01
We studied the efficiency of two different schemes for a magnetically driven quantum heat engine, by considering as the "working substance" a single nonrelativistic particle trapped in a cylindrical potential well, in the presence of an external magnetic field. The first scheme is a cycle, composed of two adiabatic and two isoenergetic reversible trajectories in configuration space. The trajectories are driven by a quasistatic modulation of the external magnetic-field intensity. The second scheme is a variant of the former, where the isoenergetic trajectories are replaced by isothermal ones, along which the system is in contact with macroscopic thermostats. This second scheme constitutes a quantum analog of the classical Carnot cycle. PMID:25353739
Pressure-Induced Magnetic Crossover Driven by Hydrogen Bonding in CuF2(H2O)2(3-chloropyridine)
O'Neal, Kenneth R.; Brinzari, Tatiana V.; Wright, Joshua B.; Ma, Chunli; Giri, Santanab; Schlueter, John A.; Wang, Qian; Jena, Puru; Liu, Zhenxian; Musfeldt, Janice L.
2014-01-01
Hydrogen bonding plays a foundational role in the life, earth, and chemical sciences, with its richness and strength depending on the situation. In molecular materials, these interactions determine assembly mechanisms, control superconductivity, and even permit magnetic exchange. In spite of its long-standing importance, exquisite control of hydrogen bonding in molecule-based magnets has only been realized in limited form and remains as one of the major challenges. Here, we report the discovery that pressure can tune the dimensionality of hydrogen bonding networks in CuF2(H2O)2(3-chloropyridine) to induce magnetic switching. Specifically, we reveal how the development of exchange pathways under compression combined with an enhanced ab-plane hydrogen bonding network yields a three dimensional superexchange web between copper centers that triggers a reversible magnetic crossover. Similar pressure- and strain-driven crossover mechanisms involving coordinated motion of hydrogen bond networks may play out in other quantum magnets. PMID:25116701
Magnetism in ultracold quantum gases
NASA Astrophysics Data System (ADS)
Schmaljohann, H.; Erhard, M.; Kronjäger, J.; Kottke, M.; van Staa, S.; Arlt, J. J.; Bongs, K.; Sengstock, K.
2004-12-01
We study the static and dynamic magnetic properties of ultracold quantum gases, in particular the spinor physics of F = 1 and F = 2 Bose-Einstein condensates of 87Rb atoms. Our data lead to the conclusion, that the F = 2 ground state of 87Rb is polar, while we find the F = 1 ground state to be ferromagnetic. The dynamics of spinor systems is linked to an interplay between coherent mean-field interactions, losses and interactions with atoms in the thermal cloud. Within this rich parameter space we observe indications for coherent spinor dynamics and novel thermalization regimes.
Annihilation of Quantum Magnetic Fluxes
NASA Astrophysics Data System (ADS)
Gonzalez, W. D.
After introducing the concepts associated with the Aharonov and Bohm effect and with the existence of a quantum of magnetic flux (QMF), we briefly discuss the Ginzburg-Landau theory that explains its origin and fundamental consequences. Also relevant observations of QMFs obtained in the laboratory using superconducting systems (vortices) are mentioned. Next, we describe processes related with the interaction of QMFs with opposite directions in terms of the gauge field geometry related to the vector potential. Then, we discuss the use of a Lagrangian density for a scalar field theory involving radiation in order to describe the annihilation of QMFs, claimed to be responsible for the emission of photons with energies corresponding to that of the annihilated magnetic fields. Finally, a possible application of these concepts to the observed variable dynamics of neutron stars is briefly mentioned.
O'Neal, Kenneth R.; Brinzari, Tatiana V.; Wright, Joshua B.; Ma, Chunli; Giri, Santanab; Schlueter, John A.; Wang, Qian; Jena, Puru; Liu, Zhenxian; Musfeldt, Janice L.
2014-08-13
Here, hydrogen bonding plays a foundational role in the life, earth, and chemical sciences, with its richness and strength depending on the situation. In molecular materials, these interactions determine assembly mechanisms, control superconductivity, and even permit magnetic exchange. In spite of its long-standing importance, exquisite control of hydrogen bonding in molecule-based magnets has only been realized in limited form and remains as one of the major challenges. Here, we report the discovery that pressure can tune the dimensionality of hydrogen bonding networks in CuF_{2}(H_{2}O)_{2}(3-chloropyridine) to induce magnetic switching. Specifically, we reveal how the development of exchange pathways under compression combined with an enhanced ab-plane hydrogen bonding network yields a three dimensional superexchange web between copper centers that triggers a reversible magnetic crossover. Similar pressure- and strain-driven crossover mechanisms involving coordinated motion of hydrogen bond networks may play out in other quantum magnets.
Pressure-induced magnetic crossover driven by hydrogen bonding in CuF2(H2O)2(3-chloropyridine)
O'Neal, Kenneth R.; Brinzari, Tatiana V.; Wright, Joshua B.; Ma, Chunli; Giri, Santanab; Schlueter, John A.; Wang, Qian; Jena, Puru; Liu, Zhenxian; Musfeldt, Janice L.
2014-08-13
Here, hydrogen bonding plays a foundational role in the life, earth, and chemical sciences, with its richness and strength depending on the situation. In molecular materials, these interactions determine assembly mechanisms, control superconductivity, and even permit magnetic exchange. In spite of its long-standing importance, exquisite control of hydrogen bonding in molecule-based magnets has only been realized in limited form and remains as one of the major challenges. Here, we report the discovery that pressure can tune the dimensionality of hydrogen bonding networks in CuF2(H2O)2(3-chloropyridine) to induce magnetic switching. Specifically, we reveal how the development of exchange pathways under compression combinedmore » with an enhanced ab-plane hydrogen bonding network yields a three dimensional superexchange web between copper centers that triggers a reversible magnetic crossover. Similar pressure- and strain-driven crossover mechanisms involving coordinated motion of hydrogen bond networks may play out in other quantum magnets.« less
Quantum information approach to the azurite mineral frustrated quantum magnet
NASA Astrophysics Data System (ADS)
Batle, J.; Ooi, C. H. Raymond; Abutalib, M.; Farouk, Ahmed; Abdalla, S.
2016-07-01
Quantum correlations are almost impossible to address in bulk systems. Quantum measures extended only to a few number of parties can be discussed in practice. In the present work, we study nonlocality for a cluster of spins belonging to a mineral whose structure is that of a quantum magnet. We reproduce at a much smaller scale the experimental outcomes, and then, we study the role of quantum correlations there. A macroscopic entanglement witness has been introduced in order to reveal nonlocal quantum correlations between individual constituents of the azurite mineral at nonzero temperatures. The critical point beyond which entanglement is zero is found at T_c < 1 K.
Quantum information approach to the azurite mineral frustrated quantum magnet
NASA Astrophysics Data System (ADS)
Batle, J.; Ooi, C. H. Raymond; Abutalib, M.; Farouk, Ahmed; Abdalla, S.
2016-04-01
Quantum correlations are almost impossible to address in bulk systems. Quantum measures extended only to a few number of parties can be discussed in practice. In the present work, we study nonlocality for a cluster of spins belonging to a mineral whose structure is that of a quantum magnet. We reproduce at a much smaller scale the experimental outcomes, and then, we study the role of quantum correlations there. A macroscopic entanglement witness has been introduced in order to reveal nonlocal quantum correlations between individual constituents of the azurite mineral at nonzero temperatures. The critical point beyond which entanglement is zero is found at T_c < 1 K.
Quantum entanglement and coherence in molecular magnets
NASA Astrophysics Data System (ADS)
Shiddiq, Muhandis
Quantum computers are predicted to outperform classical computers in certain tasks, such as factoring large numbers and searching databases. The construction of a computer whose operation is based on the principles of quantum mechanics appears extremely challenging. Solid state approaches offer the potential to answer this challenge by tailor-making novel nanomaterials for quantum information processing (QIP). Molecular magnets, which are materials whose energy levels and magnetic quantum states are well defined at the molecular level, have been identified as a class of material with properties that make them attractive for quantum computing purpose. In this dissertation, I explore the possibilities and challenges for molecular magnets to be used in quantum computing architecture. The properties of molecular magnets that are critical for applications in quantum computing, i.e., quantum entanglement and coherence, are comprehensively investigated to probe the feasibility of molecular magnets to be used as quantum bits (qubits). Interactions of qubits with photons are at the core of QIP. Photons can be used to detect and manipulate qubits, after which information can then be transferred over long distances. As a potential candidate for qubits, the interactions between Fe8 single-molecule magnets (SMMs) and cavity photons were studied. An earlier report described that a cavity mode splitting was observed in a spectrum of a cavity filled with a single-crystal of Fe8 SMMs. This splitting was interpreted as a vacuum Rabi splitting (VRS), which is a signature of an entanglement between a large number of SMMs and a cavity photon. However, find that large absorption and dispersion of the magnetic susceptibility are the reasons for this splitting. This finding highlights the fact that an observation of a peak splitting in a cavity transmission spectrum neither represents an unambiguous indication of quantum coherence in a large number of spins, nor a signature of
Quantum phase transitions in disordered magnets
NASA Astrophysics Data System (ADS)
Nozadze, David
We study the effects of quenched weak disorder on quantum phase transitions in disordered magnets. The presence of disorder in the system can lead to a variety of exotic phenomena, e.g., the smearing of transitions or quantum Griffiths singularities. Phase transitions are smeared if individual spatial regions can order independently of the bulk system. In paper I, we study smeared quantum phase transitions in binary alloys A1-xBx that are tuned by changing the composition x. We show that in this case the ordered phase is extended over all compositions x < 1. We also study the composition dependence of observables. In paper II, we investigate the influence of spatial disorder correlations on smeared phase transitions. As an experimental example, we demonstrate in paper III, that the composition-driven ferromagnetic-toparamagnetic quantum phase transition in Sr1-xCaxRuO3 is smeared. When individual spatial regions cannot order but fluctuate slowly, the phase transition is characterized by strong singularities in the quantum Griffiths phase. In paper IV, we develop a theory of the quantum Griffiths phases in disordered ferromagnetic metals. We show that the quantum Griffiths singularities are stronger than the usual power-law quantum Griffiths singularities in insulating magnets. In paper V, we present an efficient numerical method for studying quantum phase transitions in disordered systems with O(N) order parameter symmetry in the large-N limit. Our algorithm solves iteratively the large-N self-consistent equations for the renormalized distances from criticality. Paper VI is devoted to the study of transport properties in the quantum Griffiths phase associated with the antiferromagnetic quantum phase transition in a metal. We find unusual behavior of transport properties which is in contrast to the normal Fermi-liquid behavior.
NASA Astrophysics Data System (ADS)
Gui, Hong; Li, Xin; Zhao, Zhenjie; Xie, Wenhui
2016-02-01
The pressure-induced transition of Sr2FeO3 was studied by first-principle calculation using density functional theory with the generalized gradient approximation plus on-site coulomb repulsion method. It shows that Sr2FeO3 exhibits a structure transition from Immm to Ammm and at about 35 GPa and then a spin transition from high spin S = 2 to intermediate spin S = 1. And it is also revealed that the pressure leads to a change in the Fe three-dimensional electronic configuration from ({{d}{{z2}}}\\uparrow )1({{d}yz}\\uparrow )1({{d}xz}\\uparrow )1({{d}xy}\\uparrow )1({{d}{{x2}-{{y}2}}}\\uparrow )1 ({{d}{{z2}}}\\downarrow )1 under ambient conditions to ({{d}{{z2}}}\\uparrow )1({{d}yz}\\uparrow )1({{d}xz}\\uparrow )1({{d}xy}\\uparrow )1 ({{d}{{x2}-{{y}2}}}\\uparrow ) δ ({{d}yz}\\downarrow )1 ({{d}{{z2}}}\\downarrow ) σ at high pressure, where δ plus σ equals 1.
Quantum Criticality in an Organic Magnet
Stone, Matthew B; Broholm, C. L.; Reich, D. H.; Tchemyshyov, O.; Vorderwisch, P.; Harrison, N.
2006-01-01
Exchange interactions between S=1/2 sites in piperazinium hexachlorodicuprate produce a frustrated bilayer magnet with a singlet ground state. We have determined the field-temperature phase diagram by high field magnetization and neutron scattering experiments. There are two quantum critical points: H{sub c1}=7.5 T separates a quantum paramagnet phase from a three dimensional, antiferromagnetically ordered state while H{sub c2}=37 T marks the onset of a fully polarized state. The ordered phase, which we describe as a magnon Bose-Einstein condensate (BEC), is embedded in a quantum critical regime with short range correlations. A low temperature anomaly in the BEC phase boundary indicates that additional low energy features of the material become important near H{sub c1}.
Mesoscopic quantum tunneling of the magnetization
NASA Astrophysics Data System (ADS)
Barbara, B.; Wernsdorfer, W.; Sampaio, L. C.; Park, J. G.; Paulsen, C.; Novak, M. A.; Ferré, R.; Mailly, D.; Sessoli, R.; Caneschi, A.; Hasselbach, K.; Benoit, A.; Thomas, L.
1995-02-01
Magnetic relaxation plateaux observed at low temperature in complex systems, are generally attributed to Quantum Tunneling of the Magnetization (QTM). If the experiments are not performed down to low enough temperatures, alternative interpretations can be given in terms of powerlaw distributions resulting from either switching field distributions or/and coupling between switching blocks leading to self-organized criticality. Besides, the first low-temperature/time-dependent magnetization experiments, performed on single sub-micronic particles and on arrays nanoparticles in molecular crystals, are described.
Quantum transport of energy in controlled synthetic quantum magnets
NASA Astrophysics Data System (ADS)
Bermudez, Alejandro; Schaetz, Tobias
2016-08-01
We introduce a theoretical scheme that exploits laser cooling and phonon-mediated spin–spin interactions in crystals of trapped atomic ions to explore the transport of energy through a quantum magnet. We show how to implement an effective transport window to control the flow of energy through the magnet even in the absence of fermionic statistics for the carriers. This is achieved by shaping the density of states of the effective thermal reservoirs that arise from the interaction with the external bath of the modes of the electromagnetic field, and can be experimentally controlled by tuning the laser frequencies and intensities appropriately. The interplay of this transport window with the spin–spin interactions is exploited to build an analogue of the Coulomb-blockade effect in nano-scale electronic devices, and opens new possibilities to study quantum effects in energy transport.
Magnetic monopoles in quantum spin ice
NASA Astrophysics Data System (ADS)
Petrova, Olga; Moessner, Roderich; Sondhi, Shivaji
Typical spin ice materials can be modeled using classical Ising spins. The geometric frustration of the pyrochlore lattice causes the spins to satisfy ice rules, whereas a violation of the ice constraint constitutes an excitation. Flipping adjacent spins fractionalizes the excitation into two monopoles. Long range dipolar spin couplings result in Coulombic interactions between charges, while the leading effect of quantum fluctuations is to provide the monopoles with kinetic energy. We study the effect of adding quantum dynamics to spin ice, a well-known classical spin liquid, with a particular view of how to best detect its presence in experiment. For the weakly diluted quantum spin ice, we find a particularly crisp phenomenon, namely, the emergence of hydrogenic excited states in which a magnetic monopole is bound to a vacancy at various distances.
Magnetic quantum diesel engine in Ni2
NASA Astrophysics Data System (ADS)
Dong, C. D.; Lefkidis, G.; Hübner, W.
2013-12-01
Quantum Diesel cycles are numerically realized using the electronic states of a Ni2 dimer. The quantum nature and the complexity of the electronic structure of the Ni2 dimer result in new features in the evolution of the pressure as well as in the heat-work transformation. The multitude of internal degrees of freedom in the isobaric process in molecules can result in crossing of the two adiabatic processes in the P-V diagram. The interplay of heat and work, originating from thermal nonequilibrium effects, can lead to a thermal efficiency of up to 100%. The spin moment of the Ni2 can be decreased by the isobaric process. To link the molecular heat capacity to easily accessible experimental quantities, we also calculate the Kerr effect and the magnetic susceptibility at different temperatures and magnetic fields.
Towards Quantum Magnetism with Ultracold Quantum Gases in Optical Lattices
NASA Astrophysics Data System (ADS)
Bloch, Immanuel
2008-05-01
Quantum mechanical superexchange interactions form the basis of quantum magnetism in strongly correlated electronic media and are believed to play a major role in high-Tc superconducting materials. We report on the first direct measurement of such superexchange interactions with ultracold atoms in optical lattices. After preparing a spin-mixture of ultracold atoms with the help of optical superlattices in an antiferromagnetically ordered state, we are able to observe a coherent superexchange mediated spin dynamics down to coupling energies as low as 5 Hz. Furthermore, it is shown how these superexchange interactions can be fully controlled in magnitude and sign. The prospects of using such superexchange interactions for the investigation of dynamical behaviour in quantum spin systems and for quantum information processing will be outlined in the talk. In addition we present results on the dynamical resolved co-tunneling of repulsively bound atom pairs in optical superlattices and show how by using ``Coulomb-blockade'' type tunneling resonance one can count atoms one by one to determine their number statistics in the lattice potential. Finally, latest results on ultracold Fermions and Bose-Fermi mixtures in optical lattices will be presented.
Towards Quantum Magnetism with Ultracold Quantum Gases in Optical Lattices
NASA Astrophysics Data System (ADS)
Bloch, Immanuel
2008-03-01
Quantum mechanical superexchange interactions form the basis of quantum magnetism in strongly correlated electronic media and are believed to play a major role in high-Tc superconducting materials. We report on the first direct measurement of such superexchange interactions with ultracold atoms in optical lattices. After preparing a spin-mixture of ultracold atoms with the help of optical superlattices in an antiferromagnetically ordered state, we are able to observe a coherent superexchange mediated spin dynamics down to coupling energies as low as 5 Hz. Furthermore, it is shown how these superexchange interactions can be fully controlled in magnitude and sign. The prospects of using such superexchange interactions for the investigation of dynamical behaviour in quantum spin systems and for quantum information processing will be outlined in the talk. In addition we present results on the dynamical resolved co-tunnelling of repulsively bound atom pairs in optical superlattices and show how by using ``Coulomb-blockade'' type tunnelling resonance one can count atoms one by one to determine their number statistics in the lattice potential. Finally, latest results on ultracold Fermions and Bose-Fermi mixtures in optical lattices will be presented.
Quantum magnetism on kagome lattice
NASA Astrophysics Data System (ADS)
Hao, Zhihao
The spin 1/2 Heisenberg antiferromagnet on kagome (a planar lattice of corner sharing triangles) is one of the most celebrated models of a strongly correlated system. Despite intensive studies, the physics of its ground state and excitations remains unsettled. Recently, researchers successfully synthesized and characterized several new materials described by this model. It is hoped that the longstanding problem can be finally resolved through combined efforts of experimentalists, material scientists and theorists. In this thesis, we present a physical picture of the low energy physics of kagome. We demonstrate that there are N/3 fermionic particles on a kagome of N sites. The motion of these particles is strongly constrained. They are bound into small bosonic states by strong pair-wise attractions. The "antiparticle" also exists and a particle-antiparticle pair can be created at energy cost 0.218J. Low energy spin 1 excitations correspond to breaking a bound state into two free particles at energy cost 0.06J. This is the physical mechanism of the kagome spin gap. Our physical picture finds several applications. The dynamical structure factor of pair-breaking processes on kagome is computed. We assume the bound states are independent thanks to their small sizes. The result agrees well with the recent inelastic neutron scattering measurement conducted on herbertsmithite, a kagome antiferromagnet. In the second application, we study the effect of Dzyaloshinskii-Moriya (DM) interaction. DM interaction is important for low energy physics on kagome since the ground state of the dominate exchange interaction is highly degenerated. Through analytical and numerical arguments, it is determined that the vacuum become unstable to creation of particle-antiparticle pairs at critical strength D of DM interaction on the sawtooth chain, a chain of corner sharing triangles. We speculate that the mechanism is behind the numerically observed quantum phase transition at finite D on
Pressure induced magnetic phase transition in RhFe3N and IrFe3N: An ab-initio study
NASA Astrophysics Data System (ADS)
Puvaneswari, S.; Rajeswarapalanichamy, R.; Manikandan, M.
2016-05-01
The structural, electronic, elastic and magnetic properties of RhFe3N and IrFe3N are investigated using ab-initio calculations based on density functional theory as implemented in VASP code within the gradient generalized approximation. The non-spin polarized and spin polarized calculations are performed for these nitrides at normal and high pressures. It is found that these ternary nitrides are stable in ferromagnetic state at normal pressure. The lattice constant and bulk modulus values are calculated. The electronic structure reveals that these nitrides are metallic at normal pressure. The calculated elastic constants indicate that they are mechanically stable at ambient pressure. Ferromagnetic to nonmagnetic phase transition is observed in RhFe3N and IrFe3N at high pressure. Ferromagnetism is quenched in these nitrides at high pressure.
Quantum phase transitions in frustrated magnetic systems
NASA Astrophysics Data System (ADS)
Wölfle, P.; Schmitteckert, P.
2015-07-01
We review our recent work on quantum phase transitions in frustrated magnetic systems. In the first part a Pseudo Fermion Functional Renormalization Group (PFFRG) method is presented. By using an exact representation of spin 1/2 operators in terms of pseudofermions a quantum spin Hamiltonian may be mapped onto an interacting fermion system. For the latter an FRG treatment is employed. The results for the J1-J2 model and similar models of frustrated interaction show phase diagrams in agreement with those obtained by other methods, but give more detailed information on the nature of correlations, in particular in the non-magnetic phases. Applications of PFFRG to geometrically frustrated systems and to highly anisotropic Kitaev type models are also reported. In the second part the derivation of quantum spin models from the microscopic many-body Hamiltonian is discussed. The results for multiband systems with strong spin-orbit interaction encountered in the iridates class of compounds are shown to resolve some of the questions posed by experiment.
Selectivity in multiple quantum nuclear magnetic resonance
Warren, W.S.
1980-11-01
The observation of multiple-quantum nuclear magnetic resonance transitions in isotropic or anisotropic liquids is shown to give readily interpretable information on molecular configurations, rates of motional processes, and intramolecular interactions. However, the observed intensity of high multiple-quantum transitions falls off dramatically as the number of coupled spins increases. The theory of multiple-quantum NMR is developed through the density matrix formalism, and exact intensities are derived for several cases (isotropic first-order systems and anisotropic systems with high symmetry) to shown that this intensity decrease is expected if standard multiple-quantum pulse sequences are used. New pulse sequences are developed which excite coherences and produce population inversions only between selected states, even though other transitions are simultaneously resonant. One type of selective excitation presented only allows molecules to absorb and emit photons in groups of n. Coherent averaging theory is extended to describe these selective sequences, and to design sequences which are selective to arbitrarily high order in the Magnus expansion. This theory and computer calculations both show that extremely good selectivity and large signal enhancements are possible.
Javaid, Saqib; Javed Akhtar, M.
2014-07-14
We have investigated the behavior of orthoferrite LaFeO{sub 3} at ambient conditions and under pressure using DFT (generalized gradient approximation (GGA)) + U approach. Ground state electronic (band gap) and magnetic properties are considerably improved due to the Hubbard correction. Moreover, the experimentally observed pressure-driven phase transition, namely, the simultaneous occurrence of spin crossover, isostructural volume collapse, and drastic reduction in electrical resistance (electronic phase transition) is nicely described by GGA + U calculations. In particular, despite a sharp drop in resistance, a small band gap still remains in the low spin state indicating an insulator to semiconductor phase transition, in good agreement with the experiments but in contrast to GGA, which predicts metallic behavior in low spin state. We discuss the origin of variation in electronic structure of LaFeO{sub 3} in low spin state as obtained from GGA to GGA + U methods. These results emphasize the importance of correlation effects in describing the pressure-driven phase transition in LaFeO{sub 3} and other rare-earth orthoferrites.
Localized whistlers in magnetized spin quantum plasmas.
Misra, A P; Brodin, G; Marklund, M; Shukla, P K
2010-11-01
The nonlinear propagation of electromagnetic (EM) electron-cyclotron waves (whistlers) along an external magnetic field, and their modulation by electrostatic small but finite amplitude ion-acoustic density perturbations are investigated in a uniform quantum plasma with intrinsic spin of electrons. The effects of the quantum force associated with the Bohm potential and the combined effects of the classical as well as the spin-induced ponderomotive forces (CPF and SPF, respectively) are taken into consideration. The latter modify the local plasma density in a self-consistent manner. The coupled modes of wave propagation is shown to be governed by a modified set of nonlinear Schrödinger-Boussinesq-like equations which admit exact solutions in form of stationary localized envelopes. Numerical simulation reveals the existence of large-scale density fluctuations that are self-consistently created by the localized whistlers in a strongly magnetized high density plasma. The conditions for the modulational instability (MI) and the value of its growth rate are obtained. Possible applications of our results, e.g., in strongly magnetized dense plasmas and in the next generation laser-solid density plasma interaction experiments are discussed. PMID:21230601
Localized whistlers in magnetized spin quantum plasmas
NASA Astrophysics Data System (ADS)
Misra, A. P.; Brodin, G.; Marklund, M.; Shukla, P. K.
2010-11-01
The nonlinear propagation of electromagnetic (EM) electron-cyclotron waves (whistlers) along an external magnetic field, and their modulation by electrostatic small but finite amplitude ion-acoustic density perturbations are investigated in a uniform quantum plasma with intrinsic spin of electrons. The effects of the quantum force associated with the Bohm potential and the combined effects of the classical as well as the spin-induced ponderomotive forces (CPF and SPF, respectively) are taken into consideration. The latter modify the local plasma density in a self-consistent manner. The coupled modes of wave propagation is shown to be governed by a modified set of nonlinear Schrödinger-Boussinesq-like equations which admit exact solutions in form of stationary localized envelopes. Numerical simulation reveals the existence of large-scale density fluctuations that are self-consistently created by the localized whistlers in a strongly magnetized high density plasma. The conditions for the modulational instability (MI) and the value of its growth rate are obtained. Possible applications of our results, e.g., in strongly magnetized dense plasmas and in the next generation laser-solid density plasma interaction experiments are discussed.
Localized whistlers in magnetized spin quantum plasmas
Misra, A. P.; Brodin, G.; Marklund, M.; Shukla, P. K.
2010-11-15
The nonlinear propagation of electromagnetic (EM) electron-cyclotron waves (whistlers) along an external magnetic field, and their modulation by electrostatic small but finite amplitude ion-acoustic density perturbations are investigated in a uniform quantum plasma with intrinsic spin of electrons. The effects of the quantum force associated with the Bohm potential and the combined effects of the classical as well as the spin-induced ponderomotive forces (CPF and SPF, respectively) are taken into consideration. The latter modify the local plasma density in a self-consistent manner. The coupled modes of wave propagation is shown to be governed by a modified set of nonlinear Schroedinger-Boussinesq-like equations which admit exact solutions in form of stationary localized envelopes. Numerical simulation reveals the existence of large-scale density fluctuations that are self-consistently created by the localized whistlers in a strongly magnetized high density plasma. The conditions for the modulational instability (MI) and the value of its growth rate are obtained. Possible applications of our results, e.g., in strongly magnetized dense plasmas and in the next generation laser-solid density plasma interaction experiments are discussed.
Quantum transport in coupled resonators enclosed synthetic magnetic flux
NASA Astrophysics Data System (ADS)
Jin, L.
2016-07-01
Quantum transport properties are instrumental to understanding quantum coherent transport processes. Potential applications of quantum transport are widespread, in areas ranging from quantum information science to quantum engineering, and not restricted to quantum state transfer, control and manipulation. Here, we study light transport in a ring array of coupled resonators enclosed synthetic magnetic flux. The ring configuration, with an arbitrary number of resonators embedded, forms a two-arm Aharonov-Bohm interferometer. The influence of magnetic flux on light transport is investigated. Tuning the magnetic flux can lead to resonant transmission, while half-integer magnetic flux quantum leads to completely destructive interference and transmission zeros in an interferometer with two equal arms.
Quantum revivals and magnetization tunneling in effective spin systems
NASA Astrophysics Data System (ADS)
Krizanac, M.; Altwein, D.; Vedmedenko, E. Y.; Wiesendanger, R.
2016-03-01
Quantum mechanical objects or nano-objects have been proposed as bits for information storage. While time-averaged properties of magnetic, quantum-mechanical particles have been extensively studied experimentally and theoretically, experimental investigations of the real time evolution of magnetization in the quantum regime were not possible until recent developments in pump-probe techniques. Here we investigate the quantum dynamics of effective spin systems by means of analytical and numerical treatments. Particular attention is paid to the quantum revival time and its relation to the magnetization tunneling. The quantum revival time has been initially defined as the recurrence time of a total wave-function. Here we show that the quantum revivals of wave-functions and expectation values in spin systems may be quite different which gives rise to a more sophisticated definition of the quantum revival within the realm of experimental research. Particularly, the revival times for integer spins coincide which is not the case for half-integer spins. Furthermore, the quantum revival is found to be shortest for integer ratios between the on-site anisotropy and an external magnetic field paving the way to novel methods of anisotropy measurements. We show that the quantum tunneling of magnetization at avoided level crossing is coherent to the quantum revival time of expectation values, leading to a connection between these two fundamental properties of quantum mechanical spins.
Magnetic breakdown in double quantum wells
Harff, N.E. |; Simmons, J.A.; Klem, J.F.; Boebinger, G.S.; Pfeiffer, L.N.; West, K.W.
1996-08-01
The authors find that a sufficiently large perpendicular magnetic field (B{sub {perpendicular}}) causes magnetic breakdown (MB) in coupled double quantum wells (QWs) that are subject to an in-plane magnetic field (B{sub {parallel}}). B{sub {parallel}} shifts one QW dispersion curve with respect to that of the other QW, resulting in an anticrossing and an energy gap. When the gap is below the Fermi level the resulting Fermi surface (FS) consists of two components, a lens-shaped inner orbit and an hour-glass shaped outer orbit. B{sub {perpendicular}} causes Landau level formation and Shubnikov-de Haas (SdH) oscillations for each component of the FS. MB occurs when the magnetic forces from B{sub {perpendicular}} become dominant and the electrons move on free-electron circular orbits rather than on the lens and hour-glass orbits. MB is observed by identifying the peaks present in the Fourier power spectrum of the longitudinal resistance vs. 1/B{sub {perpendicular}} at constant B{sub {parallel}}, an arrangement achieved with an in-situ tilting sample holder. Results are presented for two strongly coupled GaAs/AlGaAs DQW samples.
Quantum critical state in a magnetic quasicrystal.
Deguchi, Kazuhiko; Matsukawa, Shuya; Sato, Noriaki K; Hattori, Taisuke; Ishida, Kenji; Takakura, Hiroyuki; Ishimasa, Tsutomu
2012-12-01
Quasicrystals are metallic alloys that possess long-range, aperiodic structures with diffraction symmetries forbidden to conventional crystals. Since the discovery of quasicrystals by Schechtman et al. in 1984, there has been considerable progress in resolving their geometric structure. For example, it is well known that the golden ratio of mathematics and art occurs over and over again in their crystal structure. However, the characteristic properties of the electronic states--whether they are extended as in periodic crystals or localized as in amorphous materials--are still unresolved. Here we report the first observation of quantum (T = 0) critical phenomena of the Au-Al-Yb quasicrystal--the magnetic susceptibility and the electronic specific heat coefficient arising from strongly correlated 4f electrons of the Yb atoms diverge as T→0. Furthermore, we observe that this quantum critical phenomenon is robust against hydrostatic pressure. By contrast, there is no such divergence in a crystalline approximant, a phase whose composition is close to that of the quasicrystal and whose unit cell has atomic decorations (that is, icosahedral clusters of atoms) that look like the quasicrystal. These results clearly indicate that the quantum criticality is associated with the unique electronic state of the quasicrystal, that is, a spatially confined critical state. Finally we discuss the possibility that there is a general law underlying the conventional crystals and the quasicrystals. PMID:23042414
Nuclear magnetic resonance implementation of a quantum clock synchronization algorithm
Zhang Jingfu; Long, G.C; Liu Wenzhang; Deng Zhiwei; Lu Zhiheng
2004-12-01
The quantum clock synchronization (QCS) algorithm proposed by Chuang [Phys. Rev. Lett. 85, 2006 (2000)] has been implemented in a three qubit nuclear magnetic resonance quantum system. The time difference between two separated clocks can be determined by measuring the output states. The experimental realization of the QCS algorithm also demonstrates an application of the quantum phase estimation.
Surface electromagnetic wave equations in a warm magnetized quantum plasma
Li, Chunhua; Yang, Weihong; Wu, Zhengwei; Chu, Paul K.
2014-07-15
Based on the single-fluid plasma model, a theoretical investigation of surface electromagnetic waves in a warm quantum magnetized inhomogeneous plasma is presented. The surface electromagnetic waves are assumed to propagate on the plane between a vacuum and a warm quantum magnetized plasma. The quantum magnetohydrodynamic model includes quantum diffraction effect (Bohm potential), and quantum statistical pressure is used to derive the new dispersion relation of surface electromagnetic waves. And the general dispersion relation is analyzed in some special cases of interest. It is shown that surface plasma oscillations can be propagated due to quantum effects, and the propagation velocity is enhanced. Furthermore, the external magnetic field has a significant effect on surface wave's dispersion equation. Our work should be of a useful tool for investigating the physical characteristic of surface waves and physical properties of the bounded quantum plasmas.
Lu, Dawei; Xu, Nanyang; Xu, Boruo; Li, Zhaokai; Chen, Hongwei; Peng, Xinhua; Xu, Ruixue; Du, Jiangfeng
2012-10-13
Quantum computers have been proved to be able to mimic quantum systems efficiently in polynomial time. Quantum chemistry problems, such as static molecular energy calculations and dynamical chemical reaction simulations, become very intractable on classical computers with scaling up of the system. Therefore, quantum simulation is a feasible and effective approach to tackle quantum chemistry problems. Proof-of-principle experiments have been implemented on the calculation of the hydrogen molecular energies and one-dimensional chemical isomerization reaction dynamics using nuclear magnetic resonance systems. We conclude that quantum simulation will surpass classical computers for quantum chemistry in the near future. PMID:22946038
Barocaloric effect and the pressure induced solid state refrigerator
Oliveira, N. A. de
2011-03-01
The current refrigerators are based on the heating and cooling of fluids under external pressure variation. The great inconvenience of this refrigeration technology is the damage caused to the environment by the refrigerant fluids. In this paper, we discuss the magnetic barocaloric effect, i.e., the heating or cooling of magnetic materials under pressure variation and its application in the construction of refrigerators using solid magnetic compounds as refrigerant materials and pressure as the external agent. The discussion presented in this paper points out that such a pressure induced solid state refrigerator can be very interesting because it is not harmful to the environment and can exhibit a good performance.
Magnetic resonance at the quantum limit
NASA Astrophysics Data System (ADS)
Bertet, Patrice
The detection and characterization of paramagnetic species by electron-spin resonance (ESR) spectroscopy has numerous applications in chemistry, biology, and materials science. Most ESR spectrometers rely on the inductive detection of the small microwave signals emitted by the spins during their Larmor precession into a microwave resonator in which they are embedded. Using the tools offered by circuit Quantum Electrodynamics (QED), namely high quality factor superconducting micro-resonators and Josephson parametric amplifiers that operate at the quantum limit when cooled at 20mK, we report an increase of the sensitivity of inductively detected ESR by 4 orders of magnitude over the state-of-the-art, enabling the detection of 1700 Bismuth donor spins in silicon with a signal-to-noise ratio of 1 in a single echo. We also demonstrate that the energy relaxation time of the spins is limited by spontaneous emission of microwave photons into the measurement line via the resonator, which opens the way to on-demand spin initialization via the Purcell effect. These results constitute a first step towards circuit QED experiments with magnetically coupled individual spins.
Quantum simulation of magnetic kinks with dipolar lattice gases
NASA Astrophysics Data System (ADS)
Cao, Lushuai; Yin, Xiangguo; Schmelcher, Peter
2015-05-01
We propose an effective Ising spin chain constructed with dipolar quantum gases confined in a one-dimensional optical superlattice. Mapping the motional degrees of freedom of a single particle in the lattice onto a pseudo-spin results in effective transverse and longitudinal magnetic fields. This effective Ising spin chain exhibits a quantum phase transition from a paramagnetic to a single-kink phase as the dipolar interaction increases. Particularly in the single-kink phase, a magnetic kink arises in the effective spin chain and behaves as a quasi-particle in a pinning potential exerted by the longitudinal magnetic field. Being realizable with current experimental techniques, this effective Ising chain presents a unique platform for emulating the quantum phase transition as well as the magnetic kink effects in the Ising-spin chain and enriches the toolbox for quantum emulation of spin models by ultracold quantum gases.
Tateiwa, Naoyuki; Haga, Yoshinori; Matsuda, Tatsuma D.; Fisk, Zachary
2012-01-01
A miniature ceramic anvil high pressure cell (mCAC) was earlier designed by us for magnetic measurements at pressures up to 7.6 GPa in a commercial superconducting quantum interference magnetometer [N. Tateiwa , Rev. Sci. Instrum. 82, 053906 (2011)]10.1063/1.3590745. Here, we describe methods to generate pressures above 10 GPa in the mCAC. The efficiency of the pressure generation is sharply improved when the Cu-Be gasket is sufficiently preindented. The maximum pressure for the 0.6 mm culet anvils is 12.6 GPa when the Cu-Be gasket is preindented from the initial thickness of 300–60 μm. The 0.5 mm culet anvils were also tested with a rhenium gasket. The maximum pressure attainable in the mCAC is about 13 GPa. The present cell was used to study YbCu2Si2 which shows a pressure induced transition from the non-magnetic to magnetic phases at 8 GPa. We confirm a ferromagnetic transition from the dc magnetization measurement at high pressure. The mCAC can detect the ferromagnetic ordered state whose spontaneous magnetic moment is smaller than 1 μB per unit cell. The high sensitivity for magnetic measurements in the mCAC may result from the simplicity of cell structure. The present study shows the availability of the mCAC for precise magnetic measurements at pressures above 10 GPa. PMID:22667632
Electronic Transport in Quantum Wires with Magnetic Quantum Dots in Series
NASA Astrophysics Data System (ADS)
Souma, S.; Lee, S. J.; Kim, N.; Kang, T. W.; Ihm, G.; Suzuki, A.
2002-03-01
Recent advances in nanofabrication allow microstructured magnetic potentials to be applied to ballistic electrons in high mobility two-dimensional electron gases (2DEG). Electronic transport in quantum wires with single magnetic quantum dot was studied by some of present authors [1], where the magnetic quantum dot is defined by two different magnetic fields B and B0 inside and outside the circular region, respectively. It was shown that the conductance properties depend strongly on whether B^* is parallel or antiparallel to B_0. In this work, we investigate the conductance of quantum wires with magnetic quantum dots in series. The each magnetic quantum dot is defined in the same way as the single dot case. Conductance is calculated numerically by applying the recursive Green's function method based on the lattice Hamiltonian. Our numerical results show the conductance modulation due to the presence of new types of quasi-bound states formed around multiple magnetic quantum dots. [1]H.-S. Sim, G. Ihm, N. Kim, and K. J. Chang, Phys. Rev. Lett 87, 146601 (2001)
Classical and quantum mechanical motion in magnetic fields
NASA Astrophysics Data System (ADS)
Franklin, J.; Cole Newton, K.
2016-04-01
We study the motion of a particle in a particular magnetic field configuration both classically and quantum mechanically. For flux-free radially symmetric magnetic fields defined on circular regions, we establish that particle escape speeds depend, classically, on a gauge-fixed magnetic vector potential, and we demonstrate some trajectories associated with this special type of magnetic field. Then we show that some of the geometric features of the classical trajectory (perpendicular exit from the field region, trapped and escape behavior) are reproduced quantum mechanically, using a numerical method that extends the norm-preserving Crank-Nicolson method to problems involving magnetic fields. While there are similarities between the classical trajectory and the position expectation value of the quantum-mechanical solution, there are also differences, and we demonstrate some of these.
Classical and Quantum Mechanical Motion in Magnetic Fields
NASA Astrophysics Data System (ADS)
Newton, K. Cole; Franklin, Joel
2016-03-01
We study the motion of a particle in a particular magnetic field configuration both classically and quantum mechanically. For flux-free radially symmetric magnetic fields defined on circular regions, we establish that particle escape speeds depend, classically, on a gauge-fixed magnetic vector potential, and demonstrate some trajectories associated with this special type of magnetic field. Then we show that some of the geometric features of the classical trajectory (perpendicular exit from the field region, trapped and escape behavior) are reproduced quantum mechanically using a numerical method that extends the norm-preserving Crank-Nicolson method to problems involving magnetic fields. While there are similarities between the classical trajectory and the position expectation value of the quantum mechanical solution, there are also differences, and we demonstrate some of these.
Dual trapped-ion quantum simulators: an alternative route towards exotic quantum magnets
NASA Astrophysics Data System (ADS)
Graß, Tobias; Lewenstein, Maciej; Bermudez, Alejandro
2016-03-01
We present a route towards the quantum simulation of exotic quantum magnetism in ion traps by exploiting dual relations between different spin models. Our strategy allows one to start from Hamiltonians that can be realized with current technology, while properties of an exotic dual model are inferred from measurements of non-local, string-order-like, operators. The latter can be achieved from fluorescence, or from certain spectroscopic measurements, both of which can be combined with finite-size scaling by controlling the number of ions in the dual quantum simulator. We apply this concept to propose quantum simulators of frustrated quantum magnets, and Ising models with multi-spin interactions. We test the validity of the idea by showing numerically that the predictions of an ideal dual quantum simulator are not qualitatively modified by relevant perturbations that occur naturally in the trapped-ion scenario.
Fractional quantum Hall effect in a tilted magnetic field
NASA Astrophysics Data System (ADS)
Papić, Z.
2013-06-01
We discuss the orbital effect of a tilted magnetic field on the quantum Hall effect in parabolic quantum wells. Many-body states realized at the fractional (1)/(3) and (1)/(2) filling of the second electronic subband are studied using finite-size exact diagonalization. In both cases, we obtain the phase diagram consisting of a fractional quantum Hall fluid phase that persists for moderate tilts, and eventually undergoes a direct transition to the stripe phase. It is shown that tilting of the field probes the geometrical degree of freedom of fractional quantum Hall fluids, and can be partly related to the effect of band-mass anisotropy.
Decoherence induced by magnetic impurities in a quantum hall system
Kagalovsky, V.; Chudnovskiy, A. L.
2013-04-15
Scattering by magnetic impurities is known to destroy coherence of electron motion in metals and semiconductors. We investigate the decoherence introduced in a single act of electron scattering by a magnetic impurity in a quantum Hall system. For this, we introduce a fictitious nonunitary scattering matrix for electrons that reproduces the exactly calculated scattering probabilities. The strength of decoherence is identified by the deviation of eigenvalues of the product from unity. Using the fictitious scattering matrix, we estimate the width of the metallic region at the quantum Hall effect inter-plateau transition and its dependence on the exchange coupling strength and the degree of polarization of magnetic impurities.
IR photodetector based on rectangular quantum wire in magnetic field
Jha, Nandan
2014-04-24
In this paper we study rectangular quantum wire based IR detector with magnetic field applied along the wires. The energy spectrum of a particle in rectangular box shows level repulsions and crossings when external magnetic field is applied. Due to this complex level dynamics, we can tune the spacing between any two levels by varying the magnetic field. This method allows user to change the detector parameters according to his/her requirements. In this paper, we numerically calculate the energy sub-band levels of the square quantum wire in constant magnetic field along the wire and quantify the possible operating wavelength range that can be obtained by varying the magnetic field. We also calculate the photon absorption probability at different magnetic fields and give the efficiency for different wavelengths if the transition is assumed between two lowest levels.
Magnetic quantum dots and rings in two dimensions
NASA Astrophysics Data System (ADS)
Downing, C. A.; Portnoi, M. E.
2016-07-01
We consider the motion of electrons confined to a two-dimensional plane with an externally applied perpendicular inhomogeneous magnetic field, both with and without a Coulomb potential. We find that as long as the magnetic field is slowly decaying, bound states in magnetic quantum dots are indeed possible. Several example cases of such magnetic quantum dots are considered in which one can find the eigenvalues and eigenfunctions in closed form, including two hitherto unknown quasi-exactly-solvable models treated with confluent and biconfluent Heun polynomials. It is shown how a modulation of the strength of the magnetic field can exclude magnetic vortexlike states, rotating with a certain angular momenta and possessing a definite spin orientation, from forming. This indicates one may induce localization-delocalization transitions and suggests a mechanism for spin separation.
Quantum phases in intrinsic Josephson junctions: Quantum magnetism analogy
NASA Astrophysics Data System (ADS)
Machida, Masahiko; Kobayashi, Keita; Koyama, Tomio
2013-08-01
We explore quantum phases in intrinsic Josephson junction (IJJ) stacks, whose in-plane area is so small that the capacitive coupling has a dominant role in the superconducting phase dynamics. In such cases, the effective Hamiltonian for the superconducting phase can be mapped onto that of one-dimensional ferromagnetically-interacting spin model, whose spin length S depends on the magnitude of the on-site Coulomb repulsion. The ferromagnetic model for IJJ’s prefers synchronized quantum features in contrast to the antiferromagnetically-interacting model in the conventional Josephson junction arrays.
Imaging Micrometer Scale Rock Magnetism Using a Quantum Diamond Microscope
NASA Astrophysics Data System (ADS)
Fu, R. R.; Glenn, D. R.; Le Sage, D.; Andrade Lima, E.; Weiss, B. P.; Walsworth, R. L.
2014-12-01
Optically-detected magnetometry using quantum defects in diamond, known as nitrogen-vacancy (NV) color centers, is an emerging technology that allows high sensitivity and high resolution mapping of magnetic fields. Recent measurements of live magnetotactic bacteria demonstrate that such a "quantum diamond microscope" can image individual magnetic sources with <500 nm resolution, >1 mm field-of-view, and magnetic moment sensitivity <10-16 A m2 under ambient temperatures and pressures. The unprecedented combination of spatial resolution and magnetic sensitivity of the quantum diamond microscope permits magnetic analyses of previously inaccessible geologic samples in which the regions of interest are mixed with undesirable magnetic field sources at the <<100 µm scale. Here we apply this technique to chondritic meteorites, primordial aggregates formed during the accretional phase of the solar system. These meteorites consist of fine-grained matrix mixed with chondrules and other inclusions with characteristic sizes of 0.1 - 1 mm. Each chondrule records a unique magnetic history and potentially constrains nebular magnetic fields, which likely played a key role in accretion disk dynamics. The quantum diamond microscope is unique in its ability to resolve the magnetic signal of single inclusions from surrounding material. We applied the quantum diamond microscope to a variety of natural and artificial samples. Magnetic field maps of a single chondrule from the Allende CV carbonaceous chondrite (Fig. 1) show that the strongest magnetic sources are located in its 20 μm thick rim. Magnetic field sources in the chondrule interior occur in the mesostasis as isolated 10-100 μm patches that generate magnetic fields ~10 times weaker than the rim. These maps highlight the importance of spatial resolution for paleomagnetic measurements of chondrites; lower resolution measurements would permit the nearby rim material to dominate the magnetic signal, precluding accurate recovery
NASA Astrophysics Data System (ADS)
Holovatsky, V.; Bernik, I.; Yakhnevych, M.
2016-09-01
The effect of magnetic field on electron energy spectrum, wave functions and probabilities of intraband quantum transitions in multilayered spherical quantum-dot-quantum-well (QDQW) CdSe/ZnS/CdSe/ZnS is studied. Computations are performed in the framework of the effective mass approximation and rectangular potential barriers model. The wave functions are expanded over the complete basis of functions obtained as exact solutions of the Schrodinger equation for the electron in QDQW without the magnetic field. It is shown that magnetic field takes off the spectrum degeneration with respect to the magnetic quantum number and changes the localization of electron in the nanostructure. The field stronger effects on the spherically-symmetric states, especially in the case of electron location in the outer potential well. The magnetic field changes more the radial distribution of probability of electron location in QDQW than the angular one. The oscillator strengths of intraband quantum transitions are calculated as functions of the magnetic field induction and their selection rules are established.
Magnetic torque anomaly in the quantum limit of Weyl semimetals
Moll, Philip J. W.; Potter, Andrew C.; Nair, Nityan L.; Ramshaw, B. J.; Modic, K. A.; Riggs, Scott; Zeng, Bin; Ghimire, Nirmal J.; Bauer, Eric D.; Kealhofer, Robert; Ronning, Filip; Analytis, James G.
2016-01-01
Electrons in materials with linear dispersion behave as massless Weyl- or Dirac-quasiparticles, and continue to intrigue due to their close resemblance to elusive ultra-relativistic particles as well as their potential for future electronics. Yet the experimental signatures of Weyl-fermions are often subtle and indirect, in particular if they coexist with conventional, massive quasiparticles. Here we show a pronounced anomaly in the magnetic torque of the Weyl semimetal NbAs upon entering the quantum limit state in high magnetic fields. The torque changes sign in the quantum limit, signalling a reversal of the magnetic anisotropy that can be directly attributed to the topological nature of the Weyl electrons. Our results establish that anomalous quantum limit torque measurements provide a direct experimental method to identify and distinguish Weyl and Dirac systems. PMID:27545105
Magnetic torque anomaly in the quantum limit of Weyl semimetals.
Moll, Philip J W; Potter, Andrew C; Nair, Nityan L; Ramshaw, B J; Modic, K A; Riggs, Scott; Zeng, Bin; Ghimire, Nirmal J; Bauer, Eric D; Kealhofer, Robert; Ronning, Filip; Analytis, James G
2016-01-01
Electrons in materials with linear dispersion behave as massless Weyl- or Dirac-quasiparticles, and continue to intrigue due to their close resemblance to elusive ultra-relativistic particles as well as their potential for future electronics. Yet the experimental signatures of Weyl-fermions are often subtle and indirect, in particular if they coexist with conventional, massive quasiparticles. Here we show a pronounced anomaly in the magnetic torque of the Weyl semimetal NbAs upon entering the quantum limit state in high magnetic fields. The torque changes sign in the quantum limit, signalling a reversal of the magnetic anisotropy that can be directly attributed to the topological nature of the Weyl electrons. Our results establish that anomalous quantum limit torque measurements provide a direct experimental method to identify and distinguish Weyl and Dirac systems. PMID:27545105
Quantum magnetism of alkali Rydberg atoms
NASA Astrophysics Data System (ADS)
Malinovskaya, Svetlana; Liu, Gengyuan
2016-05-01
We discuss a method to control dynamics in many-body spin states of 87Rb Rydberg atoms. The method permits excitation of cold gases and form ordered structures of alkali atoms. It makes use of a two-photon excitation scheme with circularly polarized and linearly chirped pulses. The method aims for controlled quantum state preparation in large ensembles. It is actual for experiments studding the spin hopping dynamics and realization of quantum random walks.
The quantum dusty magnetosonic solitary wave in magnetized plasma
Wang Yunliang; Qiu Hong; Wang Fengping; Lu Yanzhen; Zhou Zhongxiang
2012-01-15
The effects of quantum statistic and quantum diffraction on the weakly two-dimensional fast quantum dusty magnetosonic wave propagating perpendicular to the external magnetic field are investigated by considering the inertialess electron, inertialess ion, and inertial cold dust in the low frequency limit. A Kadomstev-Petviashvili equation is derived for the magnetosonic solitary wave by using reductive perturbation method. The results show that the amplitude of soliton increases with the increasing of quantum diffraction effects of both electrons and ions, while the amplitude of the soliton decreases with the increasing of the quantum statistic effects. By using the numerical investigations, the interaction law of the nontrivial line-solitons with rich web structure in the interaction area among the line-solitons is studied by the Wronskian determinant method, which shows that there is no exchange of the energy, the momentum, and the angular momentum in the interaction.
Simulations of magnetic field gradients due to micro-magnets on a triple quantum dot circuit
NASA Astrophysics Data System (ADS)
Poulin-Lamarre, G.; Bureau-Oxton, C.; Kam, A.; Zawadzki, P.; Studenikin, S.; Aers, G.; Pioro-Ladrière, M.; Sachrajda, A. S.
2013-12-01
To quantify the effects of local magnetic fields on triple quantum dots, the Heisenberg Hamiltonian has been diagonalized for three electrons coupled via the exchange interaction. In particular, we have investigated different geometries of micro-magnets located on top of the triple dot in order to optimize the field gradient characteristics. In this paper, we focus on two geometries which are candidates for an addressable EDSR triple quantum dot device.
Simulations of magnetic field gradients due to micro-magnets on a triple quantum dot circuit
Poulin-Lamarre, G.; Bureau-Oxton, C.; Kam, A.; Zawadzki, P.; Aers, G.; Studenikin, S.; Pioro-Ladrière, M.; Sachrajda, A. S.
2013-12-04
To quantify the effects of local magnetic fields on triple quantum dots, the Heisenberg Hamiltonian has been diagonalized for three electrons coupled via the exchange interaction. In particular, we have investigated different geometries of micro-magnets located on top of the triple dot in order to optimize the field gradient characteristics. In this paper, we focus on two geometries which are candidates for an addressable EDSR triple quantum dot device.
Nonequilibrium quantum magnetism in a dipolar lattice gas.
de Paz, A; Sharma, A; Chotia, A; Maréchal, E; Huckans, J H; Pedri, P; Santos, L; Gorceix, O; Vernac, L; Laburthe-Tolra, B
2013-11-01
We report on the realization of quantum magnetism using a degenerate dipolar gas in an optical lattice. Our system implements a lattice model resembling the celebrated t-J model. It is characterized by a nonequilibrium spinor dynamics resulting from intersite Heisenberg-like spin-spin interactions provided by nonlocal dipole-dipole interactions. Moreover, due to its large spin, our chromium lattice gases constitute an excellent environment for the study of quantum magnetism of high-spin systems, as illustrated by the complex spin dynamics observed for doubly occupied sites. PMID:24237534
Conductivity of quantum wires in uniform magnetic fields
Sinyavskii, E. P. Khamidullin, R. A.
2006-11-15
The features of the de conductivity of quantum wires in longitudinal and transverse magnetic fields are studied for degenerate and nondegenerate electron gas. The conductivity is calculated on the basis of the Kubo formalism with regard to the elastic scattering of charge carriers at long-wavelength lattice vibrations. The final theoretical results for the conductivity are compared to the experimental data. The suggested model of quantum wires allows, among other things, an interpretation of the nonmonotonic dependence of the transverse magnetoresistance on the magnetic field.
Nonequilibrium Quantum Magnetism in a Dipolar Lattice Gas
NASA Astrophysics Data System (ADS)
de Paz, A.; Sharma, A.; Chotia, A.; Maréchal, E.; Huckans, J. H.; Pedri, P.; Santos, L.; Gorceix, O.; Vernac, L.; Laburthe-Tolra, B.
2013-11-01
We report on the realization of quantum magnetism using a degenerate dipolar gas in an optical lattice. Our system implements a lattice model resembling the celebrated t-J model. It is characterized by a nonequilibrium spinor dynamics resulting from intersite Heisenberg-like spin-spin interactions provided by nonlocal dipole-dipole interactions. Moreover, due to its large spin, our chromium lattice gases constitute an excellent environment for the study of quantum magnetism of high-spin systems, as illustrated by the complex spin dynamics observed for doubly occupied sites.
Rayleigh-Taylor instability in quantum magnetized viscous plasma
Hoshoudy, G. A.
2011-09-15
Quantum effects on Rayleigh-Taylor instability of stratified viscous plasmas layer under the influence of vertical magnetic field are investigated. By linearly solving the viscous QMHD equations into normal mode, a forth-order ordinary differential equation is obtained to describe the velocity perturbation. Then the growth rate is derived for the case where a plasma with exponential density distribution is confined between two rigid planes. The results show that, the presence of vertical magnetic field beside the quantum effect will bring about more stability on the growth rate of unstable configuration for viscous plasma, which is greater than that of inviscous plasma.
Magnetic rigid rotor in the quantum regime: Theoretical toolbox
NASA Astrophysics Data System (ADS)
Rusconi, Cosimo C.; Romero-Isart, Oriol
2016-02-01
We describe the quantum dynamics of a magnetic rigid rotor in the mesoscopic scale where the Einstein-De Haas effect is predominant. In particular, we consider a single-domain magnetic nanoparticle with uniaxial anisotropy in a magnetic trap. Starting from the basic Hamiltonian of the system under the macrospin approximation, we derive a bosonized Hamiltonian describing the center-of-mass motion, the total angular momentum, and the macrospin degrees of freedom of the particle treated as a rigid body. This bosonized Hamiltonian can be approximated by a simple quadratic Hamiltonian that captures the rich physics of a nanomagnet tightly confined in position, nearly not spinning, and with its macrospin antialigned to the magnetic field. The theoretical tools derived and used here can be applied to other quantum mechanical rigid rotors.
Functional renormalization group - a new approach to frustrated quantum magnetism
NASA Astrophysics Data System (ADS)
Reuther, Johannes
The experimental and theoretical investigation of quantum spin systems has become one of the central disciplines of contemporary condensed matter physics. From an experimental viewpoint, the field has been significantly fueled by the recent synthesis of novel strongly correlated materials with exotic magnetic or quantum paramagnetic ground states. From a theoretical perspective, however, the numerical treatment of realistic models for quantum magnetism in two and three spatial dimensions still constitutes a serious challenge. This particularly applies to frustrated systems, which complicate the employment of established methods. This talk intends to propagate the pseudofermion functional renormalization group (PFFRG) as a novel approach to determine large size ground state correlations of a wide class of spin Hamiltonians. Using a diagrammatic pseudofermion representation for quantum spin models, the PFFRG performs systematic summations in all two-particle fermionic interaction channels, capturing the correct balance between classical magnetic ordering and quantum fluctuations. Numerical results for various frustrated spin models on different 2D and 3D lattices are reviewed, and benchmarked against other methods if available.
Coherent radiation by quantum dots and magnetic nanoclusters
Yukalov, V. I.; Yukalova, E. P.
2014-03-31
The assemblies of either quantum dots or magnetic nanoclusters are studied. It is shown that such assemblies can produce coherent radiation. A method is developed for solving the systems of nonlinear equations describing the dynamics of such assemblies. The method is shown to be general and applicable to systems of different physical nature. Despite mathematical similarities of dynamical equations, the physics of the processes for quantum dots and magnetic nanoclusters is rather different. In a quantum dot assembly, coherence develops due to the Dicke effect of dot interactions through the common radiation field. For a system of magnetic clusters, coherence in the spin motion appears due to the Purcell effect caused by the feedback action of a resonator. Self-organized coherent spin radiation cannot arise without a resonator. This principal difference is connected with the different physical nature of dipole forces between the objects. Effective dipole interactions between the radiating quantum dots, appearing due to photon exchange, collectivize the dot radiation. While the dipolar spin interactions exist from the beginning, yet before radiation, and on the contrary, they dephase spin motion, thus destroying the coherence of moving spins. In addition, quantum dot radiation exhibits turbulent photon filamentation that is absent for radiating spins.
Quasiparticle-continuum level repulsion in a quantum magnet
Plumb, K. W.; Hwang, Kyusung; Qiu, Y.; Harriger, Leland W.; Granroth, G. Â E.; Kolesnikov, Alexander I.; Shu, G. J.; Chou, F. C.; Rüegg, Ch.; Kim, Yong Baek; et al
2015-11-30
When the energy eigenvalues of two coupled quantum states approach each other in a certain parameter space, their energy levels repel each other and level crossing is avoided. Such level repulsion, or avoided level crossing, is commonly used to describe the dispersion relation of quasiparticles in solids. But, little is known about the level repulsion when more than two quasiparticles are present; for example, in a strongly interacting quantum system where a quasiparticle can spontaneously decay into a many-particle continuum. Here we show that even in this case level repulsion exists between a long-lived quasiparticle state and a continuum. Here,more » we observe a renormalization of the quasiparticle dispersion relation due to the presence of the continuum of multi-quasiparticle states, in our fine-resolution neutron spectroscopy study of magnetic quasiparticles in the frustrated quantum magnet BiCu2PO6.« less
Quasiparticle-continuum level repulsion in a quantum magnet
Plumb, K. W.; Hwang, Kyusung; Qiu, Y.; Harriger, Leland W.; Granroth, G. Â E.; Kolesnikov, Alexander I.; Shu, G. J.; Chou, F. C.; Rüegg, Ch.; Kim, Yong Baek; Kim, Young-June
2015-11-30
When the energy eigenvalues of two coupled quantum states approach each other in a certain parameter space, their energy levels repel each other and level crossing is avoided. Such level repulsion, or avoided level crossing, is commonly used to describe the dispersion relation of quasiparticles in solids. But, little is known about the level repulsion when more than two quasiparticles are present; for example, in a strongly interacting quantum system where a quasiparticle can spontaneously decay into a many-particle continuum. Here we show that even in this case level repulsion exists between a long-lived quasiparticle state and a continuum. Here, we observe a renormalization of the quasiparticle dispersion relation due to the presence of the continuum of multi-quasiparticle states, in our fine-resolution neutron spectroscopy study of magnetic quasiparticles in the frustrated quantum magnet BiCu_{2}PO_{6}.
Quasiparticle-continuum level repulsion in a quantum magnet
NASA Astrophysics Data System (ADS)
Plumb, K. W.; Hwang, Kyusung; Qiu, Y.; Harriger, Leland W.; Granroth, G. E.; Kolesnikov, Alexander I.; Shu, G. J.; Chou, F. C.; Rüegg, Ch.; Kim, Yong Baek; Kim, Young-June
2016-03-01
When the energy eigenvalues of two coupled quantum states approach each other in a certain parameter space, their energy levels repel each other and level crossing is avoided. Such level repulsion, or avoided level crossing, is commonly used to describe the dispersion relation of quasiparticles in solids. However, little is known about the level repulsion when more than two quasiparticles are present; for example, in a strongly interacting quantum system where a quasiparticle can spontaneously decay into a many-particle continuum. Here we show that even in this case level repulsion exists between a long-lived quasiparticle state and a continuum. In our fine-resolution neutron spectroscopy study of magnetic quasiparticles in the frustrated quantum magnet BiCu2PO6, we observe a renormalization of the quasiparticle dispersion relation due to the presence of the continuum of multi-quasiparticle states.
Magnetic Resonance Detection of Individual Proton Spins Using Quantum Reporters
NASA Astrophysics Data System (ADS)
Sushkov, A. O.; Lovchinsky, I.; Chisholm, N.; Walsworth, R. L.; Park, H.; Lukin, M. D.
2014-11-01
We demonstrate a method of magnetic resonance imaging with single nuclear-spin sensitivity under ambient conditions. Our method employs isolated electronic-spin quantum bits (qubits) as magnetic resonance "reporters" on the surface of high purity diamond. These spin qubits are localized with nanometer-scale uncertainty, and their quantum state is coherently manipulated and measured optically via a proximal nitrogen-vacancy color center located a few nanometers below the diamond surface. This system is then used for sensing, coherent coupling, and imaging of individual proton spins on the diamond surface with angstrom resolution. Our approach may enable direct structural imaging of complex molecules that cannot be accessed from bulk studies. It realizes a new platform for probing novel materials, monitoring chemical reactions, and manipulation of complex systems on surfaces at a quantum level.
FIT-MART: Quantum Magnetism with a Gentle Learning Curve
NASA Astrophysics Data System (ADS)
Engelhardt, Larry; Garland, Scott C.; Rainey, Cameron; Freeman, Ray A.
We present a new open-source software package, FIT-MART, that allows non-experts to quickly get started sim- ulating quantum magnetism. FIT-MART can be downloaded as a platform-idependent executable Java (JAR) file. It allows the user to define (Heisenberg) Hamiltonians by electronically drawing pictures that represent quantum spins and operators. Sliders are automatically generated to control the values of the parameters in the model, and when the values change, several plots are updated in real time to display both the resulting energy spectra and the equilibruim magnetic properties. Several experimental data sets for real magnetic molecules are included in FIT-MART to allow easy comparison between simulated and experimental data, and FIT-MART users can also import their own data for analysis and compare the goodness of fit for different models.
Quantum theory of spin alignment in a circular magnetic nanotube
NASA Astrophysics Data System (ADS)
Bergmann, Gerd; Thompson, Richard S.; Lu, Jia G.
2015-12-01
When electron spin and momentum couple in a solid, one generally obtains intriguing and unexpected phenomena. Metallic ferromagnetic nanotubes of cobalt with circular magnetization, which have been prepared by us and others, are a particularly interesting system. Here the spins of the conduction electrons are frustrated. They would like to align parallel to the magnetic field of the magnetization, but as the electrons move quickly around the tube the spins cannot follow the magnetization direction. In a previous short theoretical paper we solved the spin dynamics using a classical model. Here we generalize our work to a quantum mechanical model. The surprising result is that the spin of most conduction electrons is not parallel or anti-parallel to the circumferential magnetization but mostly parallel or anti-parallel to the axis of the nanotube. This result means that such a cobalt nanotube is a different ferromagnet from a cobalt film or bulk cobalt.
Herzog, F; Heedt, S; Goerke, S; Ibrahim, A; Rupprecht, B; Heyn, Ch; Hardtdegen, H; Schäpers, Th; Wilde, M A; Grundler, D
2016-02-01
We report on the magnetization of ensembles of etched quantum dots with a lateral diameter of 460 nm, which we prepared from InGaAs/InP heterostructures. The quantum dots exhibit 1/B-periodic de-Haas-van-Alphen-type oscillations in the magnetization M(B) for external magnetic fields B > 2 T, measured by torque magnetometry at 0.3 K. We compare the experimental data to model calculations assuming different confinement potentials and including ensemble broadening effects. The comparison shows that a hard wall potential with an edge depletion width of 100 nm explains the magnetic behavior. Beating patterns induced by Rashba spin-orbit interaction (SOI) as measured in unpatterned and nanopatterned InGaAs/InP heterostructures are not observed for the quantum dots. From our model we predict that signatures of SOI in the magnetization could be observed in larger dots in tilted magnetic fields. PMID:26740509
Transition metal doped semiconductor quantum dots: Optical and magnetic properties
NASA Astrophysics Data System (ADS)
Dahnovsky, Yuri; Proshchenko, Vitaly; Pimachev, Artem
We study optical and magnetic properties of CdSe and Cd-Mn-Se quantum dots (QD). We find that there are two luminescence lines, one is fast and another is slow (~1ms). With the increase of a QD diameter the slow luminescence disappears at some critical QD size, thus only one line (fast) remains. Using the SAC SI computational method we find that D = 3.2 nm and D = 2.7 nm if the Mn impurity is located inside a QD or on a QD surface, respectively. For two or four Mn atoms in the quantum dot, now absorption takes place because the transition is spin-allowed. The DFT calculations of the magnetic state reveal that it is an antiferromagnet. We also study other quantum dots such as Cd-Mn-Se, Zn-Mn-S, and Zn-Mn-Se, doped and undoped. We find the slow luminescence energies for low concentrations of Mn impurities for each QD type. The calculations indicate that two luminescence lines, fast and slow, should always take place. However for Pb-Mn-S quantum dots there are now Mn levels inside a HOMO-LUMO gap, i.e., the Mn-levels are located in a PbS conduction band. The presence of Mn dopants increases the band gap and also removes the exciton peak. This effect is different to the other quantum dots.
Magnetic resonance force microscopy and a solid state quantum computer.
Pelekhov, D. V.; Martin, I.; Suter, A.; Reagor, D. W.; Hammel, P. C.
2001-01-01
A Quantum Computer (QC) is a device that utilizes the principles of Quantum Mechanics to perform computations. Such a machine would be capable of accomplishing tasks not achievable by means of any conventional digital computer, for instance factoring large numbers. Currently it appears that the QC architecture based on an array of spin quantum bits (qubits) embedded in a solid-state matrix is one of the most promising approaches to fabrication of a scalable QC. However, the fabrication and operation of a Solid State Quantum Computer (SSQC) presents very formidable challenges; primary amongst these are: (1) the characterization and control of the fabrication process of the device during its construction and (2) the readout of the computational result. Magnetic Resonance Force Microscopy (MRFM)--a novel scanning probe technique based on mechanical detection of magnetic resonance-provides an attractive means of addressing these requirements. The sensitivity of the MRFM significantly exceeds that of conventional magnetic resonance measurement methods, and it has the potential for single electron spin detection. Moreover, the MRFM is capable of true 3D subsurface imaging. These features will make MRFM an invaluable tool for the implementation of a spin-based QC. Here we present the general principles of MRFM operation, the current status of its development and indicate future directions for its improvement.
Pressure-induced phase transition in pentacene
NASA Astrophysics Data System (ADS)
Farina, L.; Brillante, A.; Della Valle, R. G.; Venuti, E.; Amboage, M.; Syassen, K.
2003-07-01
We have recently studied two solid phases of bulk pentacene (polymorphs H and C) by means of lattice phonon Raman spectroscopy. The assignment, previously based on lattice dynamics calculations alone, is now verified by X-ray diffraction measurements, conclusively confirming the existence of both polymorphs. Furthermore, Raman phonon spectra indicate a pressure-induced phase transition where the polymorph C (lower density phase) transforms to the H form (higher density phase). The onset pressure for the phase transition is only 0.2 GPa. The phase change is irreversible.
Pressure-induced transformations in molecular crystals
Taylor, R.D.; Hearne, G.R. |; Pasternak, M.P.
1995-09-01
A review is given on the unique features of the Moessbauer spectroscopy (MS) which by virtue of the quadrupole interaction and the lattice dynamics allows one to characterize some structural properties in the pressure-induced amorphous state of molecular crystals. Experiments were performed in GeI{sub 4}, SnI{sub 4} and SnBr{sub 4} by means of {sup 119}Sn and {sup 129}I MS with pressures to 35 GPa at cryogenic temperatures using diamond anvil cells.
Large and exact quantum degeneracy in a skyrmion magnet
NASA Astrophysics Data System (ADS)
Douçot, B.; Kovrizhin, D. L.; Moessner, R.
2016-03-01
We identify a large family of ground states of a topological C PN -1 skyrmion magnet whose classical degeneracy persists to all orders in a semiclassical expansion. This goes along with an exceptional robustness of the concomitant ground-state configurations, which are not at all dressed by quantum fluctuations. We trace these twin observations back to a common root: this class of topological ground states saturates a Bogomolny inequality. A similar phenomenology occurs in high-energy physics for some field theories exhibiting supersymmetry. We propose quantum Hall ferromagnets, where these skyrmions configurations arise naturally as ground states away from integer filling, as the best available laboratory realisations.
Quantum anomalous Hall effect in magnetic topological insulators
Wang, Jing; Lian, Biao; Zhang, Shou -Cheng
2015-08-25
The search for topologically non-trivial states of matter has become an important goal for condensed matter physics. Here, we give a theoretical introduction to the quantum anomalous Hall (QAH) effect based on magnetic topological insulators in two-dimensions (2D) and three-dimensions (3D). In 2D topological insulators, magnetic order breaks the symmetry between the counter-propagating helical edge states, and as a result, the quantum spin Hall effect can evolve into the QAH effect. In 3D, magnetic order opens up a gap for the topological surface states, and chiral edge state has been predicted to exist on the magnetic domain walls. We present the phase diagram in thin films of a magnetic topological insulator and review the basic mechanism of ferromagnetic order in magnetically doped topological insulators. We also review the recent experimental observation of the QAH effect. Furthermore, we discuss more recent theoretical work on the coexistence of the helical and chiral edge states, multi-channel chiral edge states, the theory of the plateau transition, and the thickness dependence in the QAH effect.
Quantum anomalous Hall effect in magnetic topological insulators
NASA Astrophysics Data System (ADS)
Wang, Jing; Lian, Biao; Zhang, Shou-Cheng
2015-12-01
The search for topologically non-trivial states of matter has become an important goal for condensed matter physics. Here, we give a theoretical introduction to the quantum anomalous Hall (QAH) effect based on magnetic topological insulators in two-dimensions (2D) and three-dimensions (3D). In 2D topological insulators, magnetic order breaks the symmetry between the counter-propagating helical edge states, and as a result, the quantum spin Hall effect can evolve into the QAH effect. In 3D, magnetic order opens up a gap for the topological surface states, and chiral edge state has been predicted to exist on the magnetic domain walls. We present the phase diagram in thin films of a magnetic topological insulator and review the basic mechanism of ferromagnetic order in magnetically doped topological insulators. We also review the recent experimental observation of the QAH effect. We discuss more recent theoretical work on the coexistence of the helical and chiral edge states, multi-channel chiral edge states, the theory of the plateau transition, and the thickness dependence in the QAH effect.
Quantum anomalous Hall effect in magnetic topological insulators
Wang, Jing; Lian, Biao; Zhang, Shou -Cheng
2015-08-25
The search for topologically non-trivial states of matter has become an important goal for condensed matter physics. Here, we give a theoretical introduction to the quantum anomalous Hall (QAH) effect based on magnetic topological insulators in two-dimensions (2D) and three-dimensions (3D). In 2D topological insulators, magnetic order breaks the symmetry between the counter-propagating helical edge states, and as a result, the quantum spin Hall effect can evolve into the QAH effect. In 3D, magnetic order opens up a gap for the topological surface states, and chiral edge state has been predicted to exist on the magnetic domain walls. We presentmore » the phase diagram in thin films of a magnetic topological insulator and review the basic mechanism of ferromagnetic order in magnetically doped topological insulators. We also review the recent experimental observation of the QAH effect. Furthermore, we discuss more recent theoretical work on the coexistence of the helical and chiral edge states, multi-channel chiral edge states, the theory of the plateau transition, and the thickness dependence in the QAH effect.« less
Quantum holography: magnetic resonance tomography and gravitational wavelets
NASA Astrophysics Data System (ADS)
Binz, Ernst; Schempp, Walter
2000-10-01
Quantum holography is a well established theory of mathematical physics based on harmonic analysis on the Heisenberg Lie group G. The geometric quantization is performed by projectivization of the complexified coadjoint orbit picture of the unitary dual G of G in order to achieve a geometric adjustment to special relativity theory. It admits applications to various imaging modalities such as synthetic aperture radar (SAR), and most importantly for the field of non-invasive medical diagnosis, to the clinical imaging modality of magnetic resonance tomography (MRI). Quantum holography explains the quantum teleportation phenomenon through Einstein-Podolsky-Rosen (EPR) channels which is a consequence of the non-locality of quantum physics. It specifically reveals what was before unobservable in special relativity, namely the light in flight (LIF) recording processing by ultra fast laser pulse trains. Finally, it provides a Lie group theoretical approach to the Kruskal coordinatized Schwarzschild manifold of quantum cosmology with large scale applications to general relativity theory such as gravitational instanton symmetries and the theory of black holes. The direct spinorial detection of gravitational wavelets emitted by the binary radio pulsar PSR 1913+16 will also be based on the principles of quantum holography.
Yamazoe, M; Kato, T; Suzuki, K; Adachi, M; Shibayama, A; Hoshi, K; Itou, M; Tsuji, N; Sakurai, Y; Sakurai, H
2016-11-01
Spin selective magnetic hysteresis (SSMH) curves, orbital selective magnetic hysteresis (OSMH) curves and magnetic quantum number selective SSMH curves are obtained for CoFeB/MgO multilayer films by combining magnetic Compton profile measurements and superconducting quantum interference device (SQUID) magnetometer measurements. Although the SQUID magnetometer measurements do not show perpendicular magnetic anisotropy (PMA) in the CoFeB/MgO multilayer film, PMA behavior is observed in the OSMH and SSMH curves for the |m| = 2 magnetic quantum number states. These facts indicate that magnetization switching behavior is dominated by the orbital magnetization of the |m| = 2 magnetic quantum number states. PMID:27602698
Magnetic Topological Insulators and Quantum Anomalous Hall Effect
NASA Astrophysics Data System (ADS)
Kou, Xufeng
The engineering of topological surface states is a key to realize applicable devices based on topological insulators (TIs). Among various proposals, introducing magnetic impurities into TIs has been proven to be an effective way to open a surface gap and integrate additional ferromagnetism with the original topological order. In this Dissertation, we study both the intrinsic electrical and magnetic properties of the magnetic TI thin films grown by molecular beam epitaxy. By doping transition element Cr into the host tetradymite-type V-VI semiconductors, we achieve robust ferromagnetic order with a strong perpendicular magnetic anisotropy. With additional top-gating capability, we realize the electric-field-controlled ferromagnetism in the magnetic TI systems, and demonstrate such magneto-electric effects can be effectively manipulated, depending on the interplays between the band topology, magnetic exchange coupling, and structural engineering. Most significantly, we report the observation of quantum anomalous Hall effect (QAHE) in the Cr-doped (BiSb)2Te3 samples where dissipationless chiral edge conduction is realized in the macroscopic millimeter-size devices without the presence of any external magnetic field, and the stability of the quantized Hall conductance of e2/h is well-maintained as the film thickness varies across the 2D hybridization limit. With additional quantum confinement, we discover the metal-to-insulator switching between two opposite QAHE states, and reveal the universal QAHE phase diagram in the thin magnetic TI samples. In addition to the uniform magnetic TIs, we further investigate the TI/Cr-doped TI bilayer structures prepared by the modulation-doped growth method. By controlling the magnetic interaction profile, we observe the Dirac hole-mediated ferromagnetism and develop an effective way to manipulate its strength. Besides, the giant spin-orbit torque in such magnetic TI-based heterostructures enables us to demonstrate the current
Surface Induced Magnetism in Quantum Dots
Meulenberg, R W; Lee, J I
2009-08-20
The study of nanometer sized semiconductor crystallites, also known as quantum dots (QDs), has seen rapid advancements in recent years in scientific disciplines ranging from chemistry, physics, biology, materials science, and engineering. QD materials of CdSe, ZnSe, InP, as well as many others, can be prepared in the size range of 1-10 nm producing uniform, nearly monodisperse materials that are typically coated with organic molecules [1-3]. The strength of charge carrier confinement, which dictates the size-dependent properties, in these QDs depends on the nature of the material and can be correlated to the Bohr radius for the system of interest. For instance, the Bohr radius for CdSe is {approx} 5 nm, while in the more covalent structure of InP, the Bohr radius approaches {approx} 10 nm. The study of CdSe QDs has been particularly extensive during the last decade because they exhibit unique and tunable optical properties and are readily synthesized with high-crystallinity and narrow size dispersions. Although the core electronic properties of CdSe are explained in terms of the quantum confinement model, experimental efforts to elucidate the surface structure of these materials have been limited. Typically, colloidal CdSe QDs are coated with an organic surfactant, which typically consists of an organo-phosphine, -thiol, or -amine, that has the function of energetically relaxing defect states via coordination to partially coordinated surface atoms. The organic surfactant also acts to enhance carrier confinement and prevent agglomeration of the particles. Chemically, it has been shown that the bonding of the surfactant to the CdSe QD occurs through Cd atoms resulting cleavage of the Se atoms and formation of a Cd-rich (i.e. non-stoichiometric) particle [5].
Quantum tunnelling of the magnetization in a monolayer of oriented single-molecule magnets.
Mannini, M; Pineider, F; Danieli, C; Totti, F; Sorace, L; Sainctavit, Ph; Arrio, M-A; Otero, E; Joly, L; Cezar, J C; Cornia, A; Sessoli, R
2010-11-18
A fundamental step towards atomic- or molecular-scale spintronic devices has recently been made by demonstrating that the spin of an individual atom deposited on a surface, or of a small paramagnetic molecule embedded in a nanojunction, can be externally controlled. An appealing next step is the extension of such a capability to the field of information storage, by taking advantage of the magnetic bistability and rich quantum behaviour of single-molecule magnets (SMMs). Recently, a proof of concept that the magnetic memory effect is retained when SMMs are chemically anchored to a metallic surface was provided. However, control of the nanoscale organization of these complex systems is required for SMMs to be integrated into molecular spintronic devices. Here we show that a preferential orientation of Fe(4) complexes on a gold surface can be achieved by chemical tailoring. As a result, the most striking quantum feature of SMMs-their stepped hysteresis loop, which results from resonant quantum tunnelling of the magnetization-can be clearly detected using synchrotron-based spectroscopic techniques. With the aid of multiple theoretical approaches, we relate the angular dependence of the quantum tunnelling resonances to the adsorption geometry, and demonstrate that molecules predominantly lie with their easy axes close to the surface normal. Our findings prove that the quantum spin dynamics can be observed in SMMs chemically grafted to surfaces, and offer a tool to reveal the organization of matter at the nanoscale. PMID:20981008
Distributed Hybridization Model for Quantum Critical Behavior in Magnetic Quasicrystals
NASA Astrophysics Data System (ADS)
Otsuki, Junya; Kusunose, Hiroaki
2016-07-01
A quantum critical behavior of the magnetic susceptibility was observed in a quasicrystal containing ytterbium. At the same time, a mixed-valence feature of Yb ions was reported, which appears to be incompatible with the magnetic instability. We derive the magnetic susceptibility by expressing the quasiperiodicity as the distributed hybridization strength between Yb 4f and conduction electrons. Assuming a wide distribution of the hybridization strength, the most f electrons behave as renormalized paramagnetic states in the Kondo or mixed-valence regime, but a small number of f moments remain unscreened. As a result, the bulk magnetic susceptibility exhibits a nontrivial power-law-like behavior, while the average f-electron occupation is that of mixed-valence systems. This model thus resolves two contradictory properties of Yb quasicrystals.
Excitation spectra of disordered dimer magnets near quantum criticality.
Vojta, Matthias
2013-08-30
For coupled-dimer magnets with quenched disorder, we introduce a generalization of the bond-operator method, appropriate to describe both singlet and magnetically ordered phases. This allows for a numerical calculation of the magnetic excitations at all energies across the phase diagram, including the strongly inhomogeneous Griffiths regime near quantum criticality. We apply the method to the bilayer Heisenberg model with bond randomness and characterize both the broadening of excitations and the transfer of spectral weight induced by disorder. Inside the antiferromagnetic phase this model features the remarkable combination of sharp magnetic Bragg peaks and broad magnons, the latter arising from the tendency to localization of low-energy excitations. PMID:24033066
Quantum Corrections Crossover and Ferromagnetism in Magnetic Topological Insulators
Bao, Lihong; Wang, Weiyi; Meyer, Nicholas; Liu, Yanwen; Zhang, Cheng; Wang, Kai; Ai, Ping; Xiu, Faxian
2013-01-01
Revelation of emerging exotic states of topological insulators (TIs) for future quantum computing applications relies on breaking time-reversal symmetry and opening a surface energy gap. Here, we report on the transport response of Bi2Te3 TI thin films in the presence of varying Cr dopants. By tracking the magnetoconductance (MC) in a low doping regime we observed a progressive crossover from weak antilocalization (WAL) to weak localization (WL) as the Cr concentration increases. In a high doping regime, however, increasing Cr concentration yields a monotonically enhanced anomalous Hall effect (AHE) accompanied by an increasing carrier density. Our results demonstrate a possibility of manipulating bulk ferromagnetism and quantum transport in magnetic TI, thus providing an alternative way for experimentally realizing exotic quantum states required by spintronic applications. PMID:23928713
Quantum synchrotron spectra from semirelativistic electrons in teragauss magnetic fields
NASA Technical Reports Server (NTRS)
Brainerd, J. J.
1987-01-01
Synchrotron spectra are calculated from quantum electrodynamic transition rates for thermal and power-law electron distributions. It is shown that quantum effects appear in thermal spectra when the photon energy is greater than the electron temperature, and in power-law spectra when the electron energy in units of the electron rest mass times the magnetic field strength in units of the critical field strength is of order unity. These spectra are compared with spectra calculated from the ultrarelativistic approximation for synchrotron emission. It is found that the approximation for the power-law spectra is good, and the approximation for thermal spectra produces the shape of the spectrum accurately but fails to give the correct normalization. Single photon pair creation masks the quantum effects for power-law distributions, so only modifications to thermal spectra are important for gamma-ray bursts.
Uniform Doping in Quantum-Dots-Based Dilute Magnetic Semiconductor.
Saha, Avijit; Shetty, Amitha; Pavan, A R; Chattopadhyay, Soma; Shibata, Tomohiro; Viswanatha, Ranjani
2016-07-01
Effective manipulation of magnetic spin within a semiconductor leading to a search for ferromagnets with semiconducting properties has evolved into an important field of dilute magnetic semiconductors (DMS). Although a lot of research is focused on understanding the still controversial origin of magnetism, efforts are also underway to develop new materials with higher magnetic temperatures for spintronics applications. However, so far, efforts toward quantum-dots(QDs)-based DMS materials are plagued with problems of phase separation, leading to nonuniform distribution of dopant ions. In this work, we have developed a strategy to synthesize highly crystalline, single-domain DMS system starting from a small magnetic core and allowing it to diffuse uniformly inside a thick CdS semiconductor matrix and achieve DMS QDs. X-ray absorption fine structure (XAFS) spectroscopy and energy-dispersive X-ray spectroscopy-scanning transmission electron microscopy (STEM-EDX) indicates the homogeneous distribution of magnetic impurities inside the semiconductor QDs leading to superior magnetic property. Further, the versatility of this technique was demonstrated by obtaining ultra large particles (∼60 nm) with uniform doping concentration as well as demonstrating the high quality magnetic response. PMID:27295453
Permanent magnetic lattices for ultracold atoms and quantum degenerate gases
NASA Astrophysics Data System (ADS)
Ghanbari, Saeed; Kieu, Tien D.; Sidorov, Andrei; Hannaford, Peter
2006-02-01
We propose the use of periodic arrays of permanent magnetic films for producing magnetic lattices of microtraps for confining, manipulating and controlling small clouds of ultracold atoms and quantum degenerate gases. Using analytical expressions and numerical calculations we show that periodic arrays of magnetic films can produce one-dimensional (1D) and two-dimensional (2D) magnetic lattices with non-zero potential minima, allowing ultracold atoms to be trapped without losses due to spin flips. In particular, we show that two crossed layers of periodic arrays of parallel rectangular magnets plus bias fields, or a single layer of periodic arrays of square-shaped magnets with three different thicknesses plus bias fields, can produce 2D magnetic lattices of microtraps having non-zero potential minima and controllable trap depth. For arrays with micron-scale periodicity, the magnetic microtraps can have very large trap depths (~0.5 mK for the realistic parameters chosen for the 2D lattice) and very tight confinement.
Designing Frustrated Quantum Magnets with Laser-Dressed Rydberg Atoms
NASA Astrophysics Data System (ADS)
Glaetzle, Alexander W.; Dalmonte, Marcello; Nath, Rejish; Gross, Christian; Bloch, Immanuel; Zoller, Peter
2015-05-01
We show how a broad class of lattice spin-1 /2 models with angular- and distance-dependent couplings can be realized with cold alkali atoms stored in optical or magnetic trap arrays. The effective spin-1 /2 is represented by a pair of atomic ground states, and spin-spin interactions are obtained by admixing van der Waals interactions between fine-structure split Rydberg states with laser light. The strengths of the diagonal spin interactions as well as the "flip-flop," and "flip-flip" and "flop-flop" interactions can be tuned by exploiting quantum interference, thus realizing different spin symmetries. The resulting energy scales of interactions compare well with typical temperatures and decoherence time scales, making the exploration of exotic forms of quantum magnetism, including emergent gauge theories and compass models, accessible within state-of-the-art experiments.
Designing frustrated quantum magnets with laser-dressed Rydberg atoms.
Glaetzle, Alexander W; Dalmonte, Marcello; Nath, Rejish; Gross, Christian; Bloch, Immanuel; Zoller, Peter
2015-05-01
We show how a broad class of lattice spin-1/2 models with angular- and distance-dependent couplings can be realized with cold alkali atoms stored in optical or magnetic trap arrays. The effective spin-1/2 is represented by a pair of atomic ground states, and spin-spin interactions are obtained by admixing van der Waals interactions between fine-structure split Rydberg states with laser light. The strengths of the diagonal spin interactions as well as the "flip-flop," and "flip-flip" and "flop-flop" interactions can be tuned by exploiting quantum interference, thus realizing different spin symmetries. The resulting energy scales of interactions compare well with typical temperatures and decoherence time scales, making the exploration of exotic forms of quantum magnetism, including emergent gauge theories and compass models, accessible within state-of-the-art experiments. PMID:25978228
Crystallization in Ising quantum magnets and Rydberg superatoms
NASA Astrophysics Data System (ADS)
Schauss, Peter
2016-05-01
Dominating finite-range interactions in many-body systems can lead to intriguing self-ordered phases of matter. For quantum magnets, Ising models with power-law interactions are among the most elementary systems that support such phases. These models can be implemented by laser coupling ensembles of ultracold atoms to Rydberg states. In this talk, I will report on the experimental preparation of crystalline ground states of such spin systems. We observe a magnetization staircase as a function of the system size and show directly the emergence of crystalline states with vanishing susceptibility. Recent results connect these findings with the picture of Rydberg superatoms. We investigated their scalability and observed collective Rabi oscillations with the perspective of using Rydberg superatoms as collective qubits. Experiments performed at Max-Planck Institute of Quantum Optics, Garching, Germany.
Two-Electron Spherical Quantum Dot in a Magnetic Field
NASA Astrophysics Data System (ADS)
Poszwa, A.
2016-07-01
We investigate three-dimensional, two-electron quantum dots in an external magnetic field B. Due to mixed spherical and cylindrical symmetry the Schrödinger equation is not completely separable. Highly accurate numerical solutions, for a wide range of B, have been obtained by the expansion of wavefunctions in double-power series and by imposing on the radial functions appropriate boundary conditions. The asymptotic limit of a very strong magnetic field and the 2D approach have been considered. Ground state properties of the two-electron semiconductor quantum dots are investigated using both the 3D and 2D models. Theoretical calculations have been compared with recent experimental results.
Exchange interaction effects on waves in magnetized quantum plasmas
Trukhanova, Mariya Iv. Andreev, Pavel A.
2015-02-15
We have applied the many-particle quantum hydrodynamics that includes the Coulomb exchange interaction to magnetized quantum plasmas. We considered a number of wave phenomena that are affected by the Coulomb exchange interaction. Since the Coulomb exchange interaction affects the longitudinal and transverse-longitudinal waves, we focused our attention on the Langmuir waves, the Trivelpiece-Gould waves, the ion-acoustic waves in non-isothermal magnetized plasmas, the dispersion of the longitudinal low-frequency ion-acoustic waves, and low-frequency electromagnetic waves at T{sub e} ≫ T{sub i}. We have studied the dispersion of these waves and present the numeric simulation of their dispersion properties.
Magnetism in Parent Iron Chalcogenides: Quantum Fluctuations Select Plaquette Order
NASA Astrophysics Data System (ADS)
Ducatman, Samuel; Perkins, Natalia B.; Chubukov, Andrey
2012-10-01
We analyze magnetic order in Fe chalcogenide Fe1+yTe, the parent compound of the high-temperature superconductor Fe1+yTe1-xSex. Experiments show that magnetic order in this material contains components with momentum Q1=(π/2,π/2) and Q2=(π/2,-π/2) in the Fe only Brillouin zone. The actual spin order depends on the interplay between these two components. Previous works assumed that the ordered state has a single Q (either Q1 or Q2). In such a state, spins form double stripes along one of the diagonals breaking the rotational C4 symmetry. We show that quantum fluctuations actually select another order—a double Q plaquette state with equal weight of Q1 and Q2 components, which preserves C4 symmetry. We argue that the order in Fe1+yTe is determined by the competition between quantum fluctuations and magnetoelastic coupling.
NASA Astrophysics Data System (ADS)
Demić, Aleksandar; Radovanović, Jelena; Milanović, Vitomir
2016-08-01
We present a method for modeling nonparabolicity effects (NPE) in quantum nanostructures in presence of external electric and magnetic field by using second order perturbation theory. The method is applied to analysis of quantum well structure and active region of a quantum cascade laser (QCL). This model will allow us to examine the influence of magnetic field on dipole matrix element in QCL structures, which will provide a better insight to how NPE can affect the gain of QCL structures.
Single cell magnetic imaging using a quantum diamond microscope
Park, H.; Weissleder, R.; Yacoby, A.; Lukin, M. D.; Lee, H.; Walsworth, R. L.; Connolly, C. B.
2015-01-01
We apply a quantum diamond microscope to detection and imaging of immunomagnetically labeled cells. This instrument uses nitrogen-vacancy (NV) centers in diamond for correlated magnetic and fluorescence imaging. Our device provides single-cell resolution and two orders of magnitude larger field of view (~1 mm2) than previous NV imaging technologies, enabling practical applications. To illustrate, we quantify cancer biomarkers expressed by rare tumor cells in a large population of healthy cells. PMID:26098019
Exact Results in Frustrated Quantum Magnetism
NASA Astrophysics Data System (ADS)
Miyahara, Shin
Most of the exact results in frustrated spin systems have for a long time been regarded as of purely academic interest, being realized only due to the special geometry of the lattices concerned. However, recent developments in material design offer the genuine possibility of producing such exact states in real materials. In fact, the exact dimer singlet state of the two-dimensional Shastry-Sutherland model has already been found as the ground state of the quasi-two-dimensional material SrCu2(BO3)2. The cooperation between experimentalists and theorists in investigating this material has caused rapid development in the understanding of low-dimensional frustrated spin systems in general, due to the extreme utility of cases where the ground state is known exactly. This fact provides information essential to recognizing novel magnetic behavior in external magnetic fields, at finite temperatures, and in other regimes. In this chapter, we introduce spin-1 / 2 models which have an exact ground state, considering first exactly solvable spin-1 / 2 Heisenberg models, exemplified by the sawtooth-chain model, the Majumdar-Ghosh model, the two-dimensional Shastry-Sutherland model, and a frustrated ladder model. Such exact states can be realized due to special symmetries on geometrically frustrated lattices. As a second class of examples, we introduce also some exact ground states in spin-1/2 models with multiple-spin interactions.
Theory for magnetic excitations in quantum spin ice
NASA Astrophysics Data System (ADS)
Onoda, Shigeki; Datta, Trinanjan
Magnetic excitations in magnetic rare-earth pyrochlore oxides called quantum spin ice (QSI) systems such as Yb2Ti2O7, Pr2Zr2O7, and Tb2Ti2O7 have attracted great interest for possible observations of the quantum dynamics of spin ice monopoles and emergent photon excitations. However, their spectral properties remain open especially for cases relevant to experimental systems. Here, we develop a theoretical framework that incorporates gauge fluctuations into a modified gauge mean-field approach, so that it reproduces key features of recent quantum Monte-Carlo results on the double broad specific heat in the simplest QSI model and can describe a continuous growth of a coherence in gauge-field correlations on cooling down to Coulomb-phase ground states. Using this new approach, we provide a theory for magnetic neutron-scattering spectra. It is found that spin-flip exchange interactions produce dispersive QSI monopole excitations which create a particle-hole continuum neutron-scattering spectrum. Gauge fluctuations give multi-particle contributions to the spectrum, which will be possibly detected in Higgs phases.
Role of the tuning parameter at magnetic quantum phase transitions
NASA Astrophysics Data System (ADS)
Fritsch, V.; Stockert, O.; Huang, C.-L.; Bagrets, N.; Kittler, W.; Taubenheim, C.; Pilawa, B.; Woitschach, S.; Huesges, Z.; Lucas, S.; Schneidewind, A.; Grube, K.; Löhneysen, H. v.
2015-07-01
Heavy-fermion systems, with their competition between Kondo and RKKY interactions, offer a rich variety of materials that may be driven to a magnetic quantum phase transition. Quite often, a quantum critical point can be approached by chemical substitution, notably of isoelectric ligands of Ce, as in CeCu6- x Au x and CePd1- x Ni x Al. While in the former we compare pressure and concentration tuning of the magnetic structure, the latter has the additional feature of geometric frustration due to the distorted kagomé sublattice of Ce atoms in the basal plane. We further present the system CeAu2Ge2 where minor structural differences between crystals grown from Sn or Au-Ge flux lead to pronounced differences in the magnetic structure, with several field-induced phases in samples grown from Au-Ge flux. Finally, non-isoelectronic substitution of Ti by V is studied in CeTi1- x V x Ge3 where CeTiGe3 is a ferromagnet, thus allowing the study of ferromagnetic quantum criticality, a rare case for heavy-fermion systems.
Xiao, Chong; Zhang, Jiajia; Xu, Jie; Tong, Wei; Cao, Boxiao; Li, Kun; Pan, Bicai; Su, Haibin; Xie, Yi
2012-01-01
Quantum tunneling of magnetization (QTMs), stemming from their importance for understanding materials with unconventional properties, has continued to attract widespread theoretical and experimental attention. However, the observation of QTMs in the most promising candidates of molecular magnets and few iron-based compounds is limited to very low temperature. Herein, we first highlight a simple system, ultrasmall half-metallic V3O4 quantum dots, as a promising candidate for the investigation of QTMs at high temperature. The quantum superparamagnetic state (QSP) as a high temperature signature of QTMs is observed at 16 K, which is beyond absolute zero temperature and much higher than that of conventional iron-based compounds due to the stronger spin-orbital coupling of V3+ ions bringing high anisotropy energy. It is undoubtedly that this ultrasmall quantum dots, V3O4, offers not only a promising candidate for theoretical understanding of QTMs but also a very exciting possibility for computers using mesoscopic magnets. PMID:23091695
Quantum information processing by nuclear magnetic resonance spectroscopy
NASA Astrophysics Data System (ADS)
Havel, T. F.; Cory, D. G.; Lloyd, S.; Boulant, N.; Fortunato, E. M.; Pravia, M. A.; Teklemariam, G.; Weinstein, Y. S.; Bhattacharyya, A.; Hou, J.
2002-03-01
Nuclear magnetic resonance (NMR) is a direct macroscopic manifestation of the quantum mechanics of the intrinsic angular momentum of atomic nuclei. It is best known for its extraordinary range of applications, which include molecular structure determination, medical imaging, and measurements of flow and diffusion rates. Most recently, liquid-state NMR spectroscopy has been found to provide a powerful experimental tool for the development and evaluation of the coherent control techniques needed for quantum information processing. This burgeoning new interdisciplinary field has the potential to achieve cryptographic, communications, and computational feats far beyond what is possible with known classical physics. Indeed, NMR has made the demonstration of many of these feats sufficiently simple to be carried out by high school summer interns working in our laboratory (see the last two authors). In this paper the basic principles of quantum information processing by NMR spectroscopy are described, along with several illustrative experiments suitable for incorporation into the undergraduate physics curriculum. These experiments are spin-spin interferometry, an implementation of the quantum Fourier transform, and the quantum simulation of a harmonic oscillator.
Pressure-induced metallization of silane
Chen,X.; Struzhkin, V.; Song, Y.; Goncharov, A.; Ahart, M.; Liu, Z.; Mao, H.; Hemley, R.
2008-01-01
There is a great interest in electronic transitions in hydrogen-rich materials under extreme conditions. It has been recently suggested that the group IVa hydrides such as methane (CH4), silane (SiH4), and germane (GeH4) become metallic at far lower pressures than pure hydrogen at equivalent densities because the hydrogen is chemically compressed in group IVa hydride compounds. Here we report measurements of Raman and infrared spectra of silane under pressure. We find that SiH4 undergoes three phase transitions before becoming opaque at 27-30 GPa. The vibrational spectra indicate the material transforms to a polymeric (framework) structure in this higher pressure range. Room-temperature infrared reflectivity data reveal that the material exhibits Drude-like metallic behavior above 60 GPa, indicating the onset of pressure-induced metallization.
Pressure-Induced Foaming of Metals
NASA Astrophysics Data System (ADS)
García-Moreno, Francisco; Mukherjee, Manas; Jiménez, Catalina; Banhart, John
2015-05-01
Pressure-induced foaming (PIF) of metals is a foaming technique in which blowing agent free compacted metal powders are foamed. The method consists of heating hot-compacted metallic precursors to above their melting temperature under gas overpressure and foaming them by pressure release. This study focuses on PIF of Al99.7 and AlSi7 alloys under both air or Ar and overpressures up to 9 bar. In situ x-ray radioscopy allows us to follow the foaming process and to perform quantitative analyses of expansion, foam morphology, and coalescence rate. Mass spectrometry helps to identify hydrogen as the foaming gas. Adsorbates on the former powder particles are found to be the primary gas source. Various advantages of this new method are identified and discussed.
Spin jam induced by quantum fluctuations in a frustrated magnet.
Yang, Junjie; Samarakoon, Anjana; Dissanayake, Sachith; Ueda, Hiroaki; Klich, Israel; Iida, Kazuki; Pajerowski, Daniel; Butch, Nicholas P; Huang, Q; Copley, John R D; Lee, Seung-Hun
2015-09-15
Since the discovery of spin glasses in dilute magnetic systems, their study has been largely focused on understanding randomness and defects as the driving mechanism. The same paradigm has also been applied to explain glassy states found in dense frustrated systems. Recently, however, it has been theoretically suggested that different mechanisms, such as quantum fluctuations and topological features, may induce glassy states in defect-free spin systems, far from the conventional dilute limit. Here we report experimental evidence for existence of a glassy state, which we call a spin jam, in the vicinity of the clean limit of a frustrated magnet, which is insensitive to a low concentration of defects. We have studied the effect of impurities on SrCr9pGa12-9pO19 [SCGO(p)], a highly frustrated magnet, in which the magnetic Cr(3+) (s = 3/2) ions form a quasi-2D triangular system of bipyramids. Our experimental data show that as the nonmagnetic Ga(3+) impurity concentration is changed, there are two distinct phases of glassiness: an exotic glassy state, which we call a spin jam, for the high magnetic concentration region (p > 0.8) and a cluster spin glass for lower magnetic concentration (p < 0.8). This observation indicates that a spin jam is a unique vantage point from which the class of glassy states of dense frustrated magnets can be understood. PMID:26324917
Spin jam induced by quantum fluctuations in a frustrated magnet
Yang, Junjie; Samarakoon, Anjana; Dissanayake, Sachith; Ueda, Hiroaki; Klich, Israel; Iida, Kazuki; Pajerowski, Daniel; Butch, Nicholas P.; Huang, Q.; Copley, John R. D.; Lee, Seung-Hun
2015-01-01
Since the discovery of spin glasses in dilute magnetic systems, their study has been largely focused on understanding randomness and defects as the driving mechanism. The same paradigm has also been applied to explain glassy states found in dense frustrated systems. Recently, however, it has been theoretically suggested that different mechanisms, such as quantum fluctuations and topological features, may induce glassy states in defect-free spin systems, far from the conventional dilute limit. Here we report experimental evidence for existence of a glassy state, which we call a spin jam, in the vicinity of the clean limit of a frustrated magnet, which is insensitive to a low concentration of defects. We have studied the effect of impurities on SrCr9pGa12-9pO19 [SCGO(p)], a highly frustrated magnet, in which the magnetic Cr3+ (s = 3/2) ions form a quasi-2D triangular system of bipyramids. Our experimental data show that as the nonmagnetic Ga3+ impurity concentration is changed, there are two distinct phases of glassiness: an exotic glassy state, which we call a spin jam, for the high magnetic concentration region (p>0.8) and a cluster spin glass for lower magnetic concentration (p<0.8). This observation indicates that a spin jam is a unique vantage point from which the class of glassy states of dense frustrated magnets can be understood. PMID:26324917
Atomic spin chains as testing ground for quantum magnetism
NASA Astrophysics Data System (ADS)
Otte, Sander
2015-03-01
The field of quantum magnetism aims to capture the rich emergent physics that arises when multiple spins interact, in terms of elementary models such as the spin 1/2 Heisenberg chain. Experimental platforms to verify these models are rare and generally do not provide the possibility to detect spin correlations locally. In my lab we use low-temperature scanning tunneling microscopy to design and build artificial spin lattices with atomic precision. Inelastic electron tunneling spectroscopy enables us to identify the ground state and probe spin excitations as a function of system size, location inside the lattice and coupling parameter values. Two types of collective excitations that play a role in many dynamic magnetic processes are spin waves (magnons) and spinons. Our experiments enable us to study both types of excitations. First, we have been able to map the standing spin wave modes of a ferromagnetic bit of six atoms, and to determine their role in the collective reversal process of the bit (Spinelli et al., Nature Materials 2014). More recently, we have crafted antiferromagnetic spin 1/2 XXZ chains, which allow us to observe spinon excitations, as well as the stepwise transition to a fully aligned phase beyond the critical magnetic field (Toskovic et al., in preparation). These findings create a promising experimental environment for putting quantum magnetic models to the test. Research funded by NWO and FOM.
Eslami, L. Faizabadi, E.
2014-05-28
The effect of magnetic contacts on spin-dependent electron transport and spin-accumulation in a quantum ring, which is threaded by a magnetic flux, is studied. The quantum ring is made up of four quantum dots, where two of them possess magnetic structure and other ones are subjected to the Rashba spin-orbit coupling. The magnetic quantum dots, referred to as magnetic quantum contacts, are connected to two external leads. Two different configurations of magnetic moments of the quantum contacts are considered; the parallel and the anti-parallel ones. When the magnetic moments are parallel, the degeneracy between the transmission coefficients of spin-up and spin-down electrons is lifted and the system can be adjusted to operate as a spin-filter. In addition, the accumulation of spin-up and spin-down electrons in non-magnetic quantum dots are different in the case of parallel magnetic moments. When the intra-dot Coulomb interaction is taken into account, we find that the electron interactions participate in separation between the accumulations of electrons with different spin directions in non-magnetic quantum dots. Furthermore, the spin-accumulation in non-magnetic quantum dots can be tuned in the both parallel and anti-parallel magnetic moments by adjusting the Rashba spin-orbit strength and the magnetic flux. Thus, the quantum ring with magnetic quantum contacts could be utilized to create tunable local magnetic moments which can be used in designing optimized nanodevices.
Quantum engineering of spin and anisotropy in magnetic molecular junctions
Jacobson, Peter; Herden, Tobias; Muenks, Matthias; Laskin, Gennadii; Brovko, Oleg; Stepanyuk, Valeri; Ternes, Markus; Kern, Klaus
2015-01-01
Single molecule magnets and single spin centres can be individually addressed when coupled to contacts forming an electrical junction. To control and engineer the magnetism of quantum devices, it is necessary to quantify how the structural and chemical environment of the junction affects the spin centre. Metrics such as coordination number or symmetry provide a simple method to quantify the local environment, but neglect the many-body interactions of an impurity spin coupled to contacts. Here, we utilize a highly corrugated hexagonal boron nitride monolayer to mediate the coupling between a cobalt spin in CoHx (x=1,2) complexes and the metal contact. While hydrogen controls the total effective spin, the corrugation smoothly tunes the Kondo exchange interaction between the spin and the underlying metal. Using scanning tunnelling microscopy and spectroscopy together with numerical simulations, we quantitatively demonstrate how the Kondo exchange interaction mimics chemical tailoring and changes the magnetic anisotropy. PMID:26456084
Magnetic quantum coherence effect in Ni4 molecular transistors.
González, Gabriel; Leuenberger, Michael N
2014-07-01
We present a theoretical study of electron transport in Ni4 molecular transistors in the presence of Zeeman spin splitting and magnetic quantum coherence (MQC). The Zeeman interaction is extended along the leads which produces gaps in the energy spectrum which allow electron transport with spin polarized along a certain direction. We show that the coherent states in resonance with the spin up or down states in the leads induces an effective coupling between localized spin states and continuum spin states in the single molecule magnet and leads, respectively. We investigate the conductance at zero temperature as a function of the applied bias and magnetic field by means of the Landauer formula, and show that the MQC is responsible for the appearence of resonances. Accordingly, we name them MQC resonances. PMID:24918902
Quantum engineering of spin and anisotropy in magnetic molecular junctions.
Jacobson, Peter; Herden, Tobias; Muenks, Matthias; Laskin, Gennadii; Brovko, Oleg; Stepanyuk, Valeri; Ternes, Markus; Kern, Klaus
2015-01-01
Single molecule magnets and single spin centres can be individually addressed when coupled to contacts forming an electrical junction. To control and engineer the magnetism of quantum devices, it is necessary to quantify how the structural and chemical environment of the junction affects the spin centre. Metrics such as coordination number or symmetry provide a simple method to quantify the local environment, but neglect the many-body interactions of an impurity spin coupled to contacts. Here, we utilize a highly corrugated hexagonal boron nitride monolayer to mediate the coupling between a cobalt spin in CoHx (x=1,2) complexes and the metal contact. While hydrogen controls the total effective spin, the corrugation smoothly tunes the Kondo exchange interaction between the spin and the underlying metal. Using scanning tunnelling microscopy and spectroscopy together with numerical simulations, we quantitatively demonstrate how the Kondo exchange interaction mimics chemical tailoring and changes the magnetic anisotropy. PMID:26456084
Dynamics of uniform quantum gases, II: Magnetic susceptibility
NASA Astrophysics Data System (ADS)
Bosse, J.; Pathak, K. N.; Singh, G. S.
2010-03-01
A general expression for temperature-dependent magnetic susceptibility of quantum gases composed of particles possessing both charge and spin degrees of freedom has been obtained within the framework of the generalized random phase approximation. The conditions for the existence of dia-, para-, and ferro-magnetism have been analyzed in terms of a parameter involving single-particle charge and spin. The limit T→0 retrieves the expressions for the Landau and the Pauli susceptibilities for an electron gas. It is found for a Bose gas that on decreasing the temperature, it passes either through a diamagnetic incomplete Meissner-effect regime or through a paramagnetic-ferromagnetic large magnetization fluctuation regime before going to the Meissner phase at T=T.
Quantum engineering of spin and anisotropy in magnetic molecular junctions
NASA Astrophysics Data System (ADS)
Jacobson, Peter; Herden, Tobias; Muenks, Matthias; Laskin, Gennadii; Brovko, Oleg; Stepanyuk, Valeri; Ternes, Markus; Kern, Klaus
2015-10-01
Single molecule magnets and single spin centres can be individually addressed when coupled to contacts forming an electrical junction. To control and engineer the magnetism of quantum devices, it is necessary to quantify how the structural and chemical environment of the junction affects the spin centre. Metrics such as coordination number or symmetry provide a simple method to quantify the local environment, but neglect the many-body interactions of an impurity spin coupled to contacts. Here, we utilize a highly corrugated hexagonal boron nitride monolayer to mediate the coupling between a cobalt spin in CoHx (x=1,2) complexes and the metal contact. While hydrogen controls the total effective spin, the corrugation smoothly tunes the Kondo exchange interaction between the spin and the underlying metal. Using scanning tunnelling microscopy and spectroscopy together with numerical simulations, we quantitatively demonstrate how the Kondo exchange interaction mimics chemical tailoring and changes the magnetic anisotropy.
Magnetic memory of a single-molecule quantum magnet wired to a gold surface
NASA Astrophysics Data System (ADS)
Mannini, Matteo; Pineider, Francesco; Sainctavit, Philippe; Danieli, Chiara; Otero, Edwige; Sciancalepore, Corrado; Talarico, Anna Maria; Arrio, Marie-Anne; Cornia, Andrea; Gatteschi, Dante; Sessoli, Roberta
2009-03-01
In the field of molecular spintronics, the use of magnetic molecules for information technology is a main target and the observation of magnetic hysteresis on individual molecules organized on surfaces is a necessary step to develop molecular memory arrays. Although simple paramagnetic molecules can show surface-induced magnetic ordering and hysteresis when deposited on ferromagnetic surfaces, information storage at the molecular level requires molecules exhibiting an intrinsic remnant magnetization, like the so-called single-molecule magnets (SMMs). These have been intensively investigated for their rich quantum behaviour but no magnetic hysteresis has been so far reported for monolayers of SMMs on various non-magnetic substrates, most probably owing to the chemical instability of clusters on surfaces. Using X-ray absorption spectroscopy and X-ray magnetic circular dichroism synchrotron-based techniques, pushed to the limits in sensitivity and operated at sub-kelvin temperatures, we have now found that robust, tailor-made Fe4 complexes retain magnetic hysteresis at gold surfaces. Our results demonstrate that isolated SMMs can be used for storing information. The road is now open to address individual molecules wired to a conducting surface in their blocked magnetization state, thereby enabling investigation of the elementary interactions between electron transport and magnetism degrees of freedom at the molecular scale.
Magnetic memory of a single-molecule quantum magnet wired to a gold surface.
Mannini, Matteo; Pineider, Francesco; Sainctavit, Philippe; Danieli, Chiara; Otero, Edwige; Sciancalepore, Corrado; Talarico, Anna Maria; Arrio, Marie-Anne; Cornia, Andrea; Gatteschi, Dante; Sessoli, Roberta
2009-03-01
In the field of molecular spintronics, the use of magnetic molecules for information technology is a main target and the observation of magnetic hysteresis on individual molecules organized on surfaces is a necessary step to develop molecular memory arrays. Although simple paramagnetic molecules can show surface-induced magnetic ordering and hysteresis when deposited on ferromagnetic surfaces, information storage at the molecular level requires molecules exhibiting an intrinsic remnant magnetization, like the so-called single-molecule magnets (SMMs). These have been intensively investigated for their rich quantum behaviour but no magnetic hysteresis has been so far reported for monolayers of SMMs on various non-magnetic substrates, most probably owing to the chemical instability of clusters on surfaces. Using X-ray absorption spectroscopy and X-ray magnetic circular dichroism synchrotron-based techniques, pushed to the limits in sensitivity and operated at sub-kelvin temperatures, we have now found that robust, tailor-made Fe(4) complexes retain magnetic hysteresis at gold surfaces. Our results demonstrate that isolated SMMs can be used for storing information. The road is now open to address individual molecules wired to a conducting surface in their blocked magnetization state, thereby enabling investigation of the elementary interactions between electron transport and magnetism degrees of freedom at the molecular scale. PMID:19182788
Suzuki, Kosuke Takubo, Shota; Kato, Tadashi; Yamazoe, Masatoshi; Hoshi, Kazushi; Sakurai, Hiroshi; Homma, Yoshiya; Itou, Masayoshi; Sakurai, Yoshiharu
2014-08-18
A spin specific magnetic hysteresis (SSMH) curve and an orbital specific magnetic hysteresis (OSMH) curve are obtained for Fe/Au/Fe/MgO multilayers by magnetic Compton scattering and SQUID magnetometer measurements. The SSMH curve with each contribution of magnetic quantum number |m| = 0, 1, and 2 states is obtained by decomposition analyses of magnetic Compton profiles. Residual magnetization is observed for the SSMH curve with magnetic quantum number |m| = 0, 2 and the OSMH curve. Although the SQUID magnetometer measurements do not show perpendicular magnetic anisotropy (PMA) in the present Fe/Au/Fe/MgO multilayer film, the SSMH curve with magnetic quantum number |m| = 0, 2 and OSMH curve show switching behaviors of PMA.
Enhanced current injection from a quantum well to a quantum dash in magnetic field
NASA Astrophysics Data System (ADS)
Paravicini-Bagliani, Gian L.; Liverini, Valeria; Valmorra, Federico; Scalari, Giacomo; Gramm, Fabian; Faist, Jérôme
2014-08-01
Resonant tunneling injection is a key ingredient in achieving population inversion in a putative quantum dot cascade laser. In a quantum dot based structure, such resonant current requires a matching of the wavefunction shape in k-space between the injector and the quantum dot. We show experimentally that the injection into an excited state of a dash structure can be enhanced tenfold by an in-plane magnetic field that shifts the injector distribution in k-space. These experiments, performed on resonant tunneling diode structures, show unambiguously resonant tunneling into an ensemble of InAs dashes grown between two AlInAs barrier layers. They also show that interface roughness scattering can enhance the tunneling current.
Transverse quantum Stern-Gerlach magnets for electrons
NASA Astrophysics Data System (ADS)
McGregor, Scot; Bach, Roger; Batelaan, Herman
2011-06-01
In the Stern-Gerlach experiment, silver atoms were separated according to their spin state (Gerlach and Stern 1922 Z. Phys. 9 353-355). This experiment demonstrates the quantization of spin and relies on the classical description of motion. However, so far, no design has led to a functional Stern-Gerlach magnet for free electrons. Bohr and Pauli showed in the 1930 Solvay conference that Stern-Gerlach magnets for electrons cannot work, at least if the design is based on classical trajectories (Pauli W 1932 Proc. of the 6th Solvay Conf. 2 (1930) (Brussels: Gauthier-Villars) pp 183-86, 217-20, 275-80 Pauli W 1964 Collected Scientific Papers ed R Kronig and V F Weiskopf, vol 2 (New York: Wiley)). Here, we present ideas for the realization of a Stern-Gerlach magnet for electrons in which spin and motion are treated fully quantum mechanically. We show that a magnetic phase grating composed of a regular array of microscopic current loops can separate electron diffraction peaks according to their spin states. The experimental feasibility of a diffractive approach is compared to that of an interferometric approach. We show that an interferometric arrangement with magnetic phase control is the functional equivalent of an electron Stern-Gerlach magnet.
Quantum spin ice: a search for gapless quantum spin liquids in pyrochlore magnets.
Gingras, M J P; McClarty, P A
2014-05-01
The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare-earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Spin ices provide one of very few experimentally realized examples of fractionalization because their elementary excitations can be regarded as magnetic monopoles and, over some temperature range, spin ice materials are best described as liquids of these emergent charges. In the presence of quantum fluctuations, one can obtain, in principle, a quantum spin liquid descended from the classical spin ice state characterized by emergent photon-like excitations. Whereas in classical spin ices the excitations are akin to electrostatic charges with a mutual Coulomb interaction, in the quantum spin liquid these charges interact through a dynamic and emergent electromagnetic field. In this review, we describe the latest developments in the study of such a quantum spin ice, focusing on the spin liquid phenomenology and the kinds of materials where such a phase might be found. PMID:24787264
Quantum Simulation of Frustrated Magnetism with Many Trapped Ions
NASA Astrophysics Data System (ADS)
Senko, Crystal
2013-05-01
A collection of trapped atomic ions is an excellent system for simulating quantum many-body physics, like magnetism, which may be difficult to access via classical computation or traditional condensed-matter experiments. Our large crystals of 10-20 ions comprise a platform to study a long-range quantum Ising model with tunable couplings in a 1D spin chain. State-dependent optical dipole forces exploit the Coulomb interaction to generate the spin-spin couplings, and fluorescence measurements on a camera are used to read out individual spin states. We investigated the spin order resulting from changing the range of antiferromagnetic interactions or the strength of an axial magnetic field, demonstrating our control over the amount of frustration present. We are turning to the study of dynamics in this system, with the aim of exploring topics including adiabaticity, spectroscopy of the Hamiltonian, the emergence of Kibble-Zurek-like behavior in a finite system, thermalization in an isolated quantum system, and nonequilibrium phase transitions. There is great promise in extending the system to 30+ spins, where computations become classically intractable. Co-authors are R. Islam, P. Richerme, W. C. Campbell, S. Korenblit, J. Smith, A. Lee, E. E. Edwards, C.-C. J. Wang, J. K. Freericks, and C. Monroe. This work is supported by grants from the U.S. Army Research Office with funding from the DARPA OLE program, IARPA, and the MURI program; and the NSF Physics Frontier Center at JQI.
Temperature and pressure-induced valence transitions in YbNi2Ge2 and YbPd2Si2
NASA Astrophysics Data System (ADS)
Yamaoka, Hitoshi; Jarrige, Ignace; Tsujii, Naohito; Lin, Jung-Fu; Hiraoka, Nozomu; Ishii, Hirofumi; Tsuei, Ku-Ding
2010-07-01
We have measured the temperature and pressure-induced Yb valence transitions in tetragonal YbNi2Ge2 and YbPd2Si2 using x-ray absorption spectroscopy in the partial fluorescence yield mode and resonant x-ray emission spectroscopy. A temperature dependence of the Yb valence on the order of 0.1 has been measured, consistent with the magnetic-susceptibility study. The crossover from the low-temperature state having a stronger mixed valence to a high-temperature local moment behavior is analyzed within the Anderson impurity model. Pressure-induced second-order valence transitions are observed for both compounds with a more gradual transition in YbPd2Si2 than that of YbNi2Ge2 . The mean valences are slightly less than 3+ at ambient pressure but increase with applying pressure. Small variations in the Yb valence on the order of 0.03-0.05 can result in drastic change in the physical properties such as magnetic order and transport properties. Our results show that the Yb valence is noninteger around the quantum critical point.
Externally controlled local magnetic field in a conducting mesoscopic ring coupled to a quantum wire
Maiti, Santanu K.
2015-01-14
In the present work, the possibility of regulating local magnetic field in a quantum ring is investigated theoretically. The ring is coupled to a quantum wire and subjected to an in-plane electric field. Under a finite bias voltage across the wire a net circulating current is established in the ring which produces a strong magnetic field at its centre. This magnetic field can be tuned externally in a wide range by regulating the in-plane electric field, and thus, our present system can be utilized to control magnetic field at a specific region. The feasibility of this quantum system in designing spin-based quantum devices is also analyzed.
Electronic Magnetization of a Quantum Point Contact Measured by Nuclear Magnetic Resonance
NASA Astrophysics Data System (ADS)
Kawamura, Minoru; Ono, Keiji; Stano, Peter; Kono, Kimitoshi; Aono, Tomosuke
2015-07-01
We report an electronic magnetization measurement of a quantum point contact (QPC) based on nuclear magnetic resonance (NMR) spectroscopy. We find that NMR signals can be detected by measuring the QPC conductance under in-plane magnetic fields. This makes it possible to measure, from Knight shifts of the NMR spectra, the electronic magnetization of a QPC containing only a few electron spins. The magnetization changes smoothly with the QPC potential barrier height and peaks at the conductance plateau of 0.5 ×2 e2/h . The observed features are well captured by a model calculation assuming a smooth potential barrier, supporting a no bound state origin of the 0.7 structure.
The quantum needle of the avian magnetic compass.
Hiscock, Hamish G; Worster, Susannah; Kattnig, Daniel R; Steers, Charlotte; Jin, Ye; Manolopoulos, David E; Mouritsen, Henrik; Hore, P J
2016-04-26
Migratory birds have a light-dependent magnetic compass, the mechanism of which is thought to involve radical pairs formed photochemically in cryptochrome proteins in the retina. Theoretical descriptions of this compass have thus far been unable to account for the high precision with which birds are able to detect the direction of the Earth's magnetic field. Here we use coherent spin dynamics simulations to explore the behavior of realistic models of cryptochrome-based radical pairs. We show that when the spin coherence persists for longer than a few microseconds, the output of the sensor contains a sharp feature, referred to as a spike. The spike arises from avoided crossings of the quantum mechanical spin energy-levels of radicals formed in cryptochromes. Such a feature could deliver a heading precision sufficient to explain the navigational behavior of migratory birds in the wild. Our results (i) afford new insights into radical pair magnetoreception, (ii) suggest ways in which the performance of the compass could have been optimized by evolution, (iii) may provide the beginnings of an explanation for the magnetic disorientation of migratory birds exposed to anthropogenic electromagnetic noise, and (iv) suggest that radical pair magnetoreception may be more of a quantum biology phenomenon than previously realized. PMID:27044102
NASA Astrophysics Data System (ADS)
Mitra, Avik; Sivapriya, K.; Kumar, Anil
2007-08-01
In a three player quantum 'Dilemma' game each player takes independent decisions to maximize his/her individual gain. The optimal strategy in the quantum version of this game has a higher payoff compared to its classical counterpart. However, this advantage is lost if the initial qubits provided to the players are from a noisy source. We have experimentally implemented the three player quantum version of the 'Dilemma' game as described by Johnson, [N.F. Johnson, Phys. Rev. A 63 (2001) 020302(R)] using nuclear magnetic resonance quantum information processor and have experimentally verified that the payoff of the quantum game for various levels of corruption matches the theoretical payoff.
Magnetic field induced minigap in double quantum wells
Simmons, J.A.; Lyo, S.K.; Klem, J.F.; Harff, N.E. |
1994-07-01
We report discovery of a partial energy gap, or minigap, in strongly coupled double quantum wells (QWs), due to an anticrossing of the two QW dispersion curves. The anticrossing and minigap are induced by an in-plane magnetic field B{sub {parallel}}, and give rise to large distortions in the Fermi surface and density of states, including a Van Hove singularity. Sweeping B{sub {parallel}} moves the minigap through the Fermi level, with the upper and lower gap edges producing a sharp maximum and minimum in the low-temperature in-plane conductance, in agreement with theoretical calculations. The gap energy may be directly determined from the data.
Magnetotransport in Dirac semimetals: Chiral magnetic effect and quantum oscillations
NASA Astrophysics Data System (ADS)
Monteiro, Gustavo; Abanov, Alexander; Kharzeev, Dmitri
Dirac semimetals are characterized by the linear dispersion of fermionic quasiparticles, with the Dirac point hidden inside a Fermi surface. We study the magnetotransport in these materials using chiral kinetic theory to describe within the same framework both the negative magnetoresistance caused by the chiral magnetic effect and quantum oscillations in the magnetoresistance due to the existence of the Fermi surface. We also consider the role of Fermi Arcs and their contribution for the SdH modes. We discuss the relevance of obtained results to recent measurements on Cd3 As2 .
Electron spin coherence near room temperature in magnetic quantum dots.
Moro, Fabrizio; Turyanska, Lyudmila; Wilman, James; Fielding, Alistair J; Fay, Michael W; Granwehr, Josef; Patanè, Amalia
2015-01-01
We report on an example of confined magnetic ions with long spin coherence near room temperature. This was achieved by confining single Mn(2+) spins in colloidal semiconductor quantum dots (QDs) and by dispersing the QDs in a proton-spin free matrix. The controlled suppression of Mn-Mn interactions and minimization of Mn-nuclear spin dipolar interactions result in unprecedentedly long phase memory (TM ~ 8 μs) and spin-lattice relaxation (T1 ~ 10 ms) time constants for Mn(2+) ions at T = 4.5 K, and in electron spin coherence observable near room temperature (TM ~ 1 μs). PMID:26040432
Spectrum of a magnetized strong-leg quantum spin ladder.
Schmidiger, D; Bouillot, P; Guidi, T; Bewley, R; Kollath, C; Giamarchi, T; Zheludev, A
2013-09-01
Inelastic neutron scattering is used to measure the spin excitation spectrum of the Heisenberg S=1/2 ladder material (C7H10N)2CuBr4 in its entirety, both in the gapped spin liquid and the magnetic field-induced Tomonaga-Luttinger spin liquid regimes. A fundamental change of the spin dynamics is observed between these two regimes. Density matrix renormalization group calculations quantitatively reproduce and help understand the observed commensurate and incommensurate excitations. The results validate long-standing quantum field-theoretical predictions but also test the limits of that approach. PMID:25166704
Magnetic phase diagram of ν=2 quantum Hall systems
NASA Astrophysics Data System (ADS)
Yoshizawa, Kanako; Takayanagi, Kazuo
2009-03-01
We present the magnetic phase diagram of the ν=2 quantum Hall system on the whole (rs,EZ) plane. We fix the phase boundaries of the paramagnetic and ferromagnetic states by looking for a softening of spin-density excitations in the time-dependent Hartree-Fock theory. A nontrivial phase is obtained in the self-consistent Hartree-Fock theory for rs˜2 and EZ≲0.06ℏωc , where both the paramagnetic and ferromagnetic states show spin instability. We show that the obtained phase is the spin-density wave (SDW) state, and explain the mechanism how the SDW stabilizes.
NASA Astrophysics Data System (ADS)
Huang, Chun-Feng; Tsai, I.-H.
It is well-established how the quantum interference induces strong localization leading to quantum Hall effect at high enough magnetic fields. Decreasing the magnetic fields, however, the localization strength can be reduced and the semiclassical magneto-oscillations following Shubnikov-de Haas formula appear in most quantum Hall systems. To understand the transport properties as the localization strength becomes weak, our team has investigated the magneto-resistance in some quantum Hall systems at low magnetic fields. Under the semiclassical transport, the crossing points in Hall plateaus showed Landau-band quantization and microwave-induced heating demonstrated the band-edge equivalence important to Landau-level addition transformation. We note that such equivalence is consistent with the edge universality based on the random matrices of Wigner type, and the Landau-band quantization can be explained by considering geometric phase effects. From our study, some quantum Hall features can survive as the semiclassical transport reveals the insufficient localization.
Tunable indirect magnetic interaction mediated by spin-orbit coupled electrons in quantum well
NASA Astrophysics Data System (ADS)
Sun, Yi-Qian; Lyu, Pin
2015-01-01
By taking into account the quantum confinement, we calculated the Ruderman-Kittel-Kasuya-Yosida (RKKY) magnetic interaction between two magnetic impurities mediated by electrons with Rashba and Dresselhaus spin-orbit couplings in a quantum well. The RKKY magnetic interaction of the present system consists of conventional RKKY magnetic coupling, anisotropic magnetic couplings and Dzyaloshinsky-Moriya magnetic interaction. The above magnetic interactions strongly depend not only on the spin-orbit coupling strength, but also on the confined width and the absolute positions of two localized spins in the direction perpendicular to the plane of the layered structure due to the quantum size effect. It provides a potential way to control the RKKY magnetic interaction and its components in the quantum well with Rashba spin-orbit coupling by both the applied gate voltage and the nanostructure geometry.
Trichoscopy of Noncicatricial Pressure-induced Alopecia Resembling Alopecia Areata
Papaiordanou, Francine; da Silveira, Bruno Rebelo Lages; Piñeiro-Maceira, Juan; Pirmez, Rodrigo
2016-01-01
Pressure-induced alopecia is an unusual cause of hair loss, and reports of its trichoscopic features are scarce. In this paper, we describe a case of pressure-induced alopecia in which trichoscopic and histopathological findings overlap with those described for alopecia areata. PMID:27601865
Trichoscopy of Noncicatricial Pressure-induced Alopecia Resembling Alopecia Areata.
Papaiordanou, Francine; da Silveira, Bruno Rebelo Lages; Piñeiro-Maceira, Juan; Pirmez, Rodrigo
2016-01-01
Pressure-induced alopecia is an unusual cause of hair loss, and reports of its trichoscopic features are scarce. In this paper, we describe a case of pressure-induced alopecia in which trichoscopic and histopathological findings overlap with those described for alopecia areata. PMID:27601865
Quantum tunneling of the magnetic moment in the S/F/S Josephson φ0 junction
NASA Astrophysics Data System (ADS)
Chudnovsky, Eugene M.
2016-04-01
We show that the S/F/S Josephson φ0 junction permits detection of macroscopic quantum tunneling and quantum oscillation of the magnetic moment by measuring the ac voltage across the junction. Exact expression for the tunnel splitting renormalized by the interaction with the superconducting order parameter is obtained. It is demonstrated that magnetic tunneling may become frozen at a sufficiently large φ0. The quality factor of quantum oscillations of the magnetic moment due to finite ohmic resistance of the junction is computed. It is shown that magnetic tunneling rate in the φ0 junction can be controlled by the bias current, with no need for the magnetic field.
Magnetic edge states in Aharonov-Bohm graphene quantum rings
NASA Astrophysics Data System (ADS)
Farghadan, R.; Saffarzadeh, A.; Heidari Semiromi, E.
2013-12-01
The effect of electron-electron interaction on the electronic structure of Aharonov-Bohm (AB) graphene quantum rings (GQRs) is explored theoretically using the single-band tight-binding Hamiltonian and the mean-field Hubbard model. The electronic states and magnetic properties of hexagonal, triangular, and circular GQRs with different sizes and zigzag edge terminations are studied. The results show that, although the AB oscillations in the all types of nanoring are affected by the interaction, the spin splitting in the AB oscillations strongly depends on the geometry and the size of graphene nanorings. We found that the total spin of hexagonal and circular rings is zero and therefore, no spin splitting can be observed in the AB oscillations. However, the non-zero magnetization of the triangular rings breaks the degeneracy between spin-up and spin-down electrons, which produces spin-polarized AB oscillations.
Quantum electrodynamical corrections to a magnetic dipole in general relativity
NASA Astrophysics Data System (ADS)
Pétri, J.
2016-03-01
Magnetized neutron stars are privileged places where strong electromagnetic fields as high as BQ = 4.4 × 109 T exist, giving rise to non-linear corrections to Maxwell equations described by quantum electrodynamics (QED). These corrections need to be included to the general relativistic (GR) description of a magnetic dipole supposed to be anchored in the neutron star. In this paper, these QED and GR perturbations to the standard flat space-time dipole are calculated to the lowest order in the fine structure constant αsf and to any order in the ratio Rs/R where R is the neutron star radius and Rs its Schwarzschild radius. Following our new 3+1 formalism developed in a previous work, we compute the multipolar non-linear corrections to this dipole and demonstrate the presence of a small dipolar ℓ = 1 and hexapolar ℓ = 3 component.
Magnetic quantum well states in ultrathin film and wedge structures
Li, D.; Bader, S.D.
1996-04-01
Magnetic quantum-well (QW) states are probed with angle- and spin-resolved photoemission to address critical issues pertaining to the origin of the giant magnetoresistance (GMR) optimization and oscillatory coupling of magnetic multilayers. Two epitaxial systems are highlighted: Cu/Co(wedge)/Cu(100) and Cr/Fe(100)-whisker. The confinement of Cu sp-QW states by a Co barrier requires a characteristic Co thickness of 2.2 {+-} 0.6 {angstrom}, which is consistent with the interfacial Co thickness reported to optimize the GMR of permalloy-Cu structures. The controversial k-space origin of the 18-{angstrom} long period oscillation in Fe/Cr multilayers is identified by the vector that spans the d-derived lens feature of the Cr Fermi surface, based on the emergence of QW states with 17 {+-} 2 {angstrom} periodicity in this region.
Ma, Minjie; Jalil, Mansoor Bin Abdul; Tan, Seng Gee
2013-03-15
The spin-dependent transport through a diluted magnetic semiconductor quantum dot (QD) which is coupled via magnetic tunnel junctions to two ferromagnetic leads is studied theoretically. A noncollinear system is considered, where the QD is magnetized at an arbitrary angle with respect to the leads' magnetization. The tunneling current is calculated in the coherent regime via the Keldysh nonequilibrium Green's function (NEGF) formalism, incorporating the electron-electron interaction in the QD. We provide the first analytical solution for the Green's function of the noncollinear DMS quantum dot system, solved via the equation of motion method under Hartree-Fock approximation. The transport characteristics (charge and spin currents, and tunnel magnetoresistance (TMR)) are evaluated for different voltage regimes. The interplay between spin-dependent tunneling and single-charge effects results in three distinct voltage regimes in the spin and charge current characteristics. The voltage range in which the QD is singly occupied corresponds to the maximum spin current and greatest sensitivity of the spin current to the QD magnetization orientation. The QD device also shows transport features suitable for sensor applications, i.e., a large charge current coupled with a high TMR ratio. - Highlights: Black-Right-Pointing-Pointer The spin polarized transport through a diluted magnetic quantum dot is studied. Black-Right-Pointing-Pointer The model is based on the Green's function and the equation of motion method. Black-Right-Pointing-Pointer The charge and spin currents and tunnel magnetoresistance (TMR) are investigated. Black-Right-Pointing-Pointer The system is suitable for current-induced spin-transfer torque application. Black-Right-Pointing-Pointer A large tunneling current and a high TMR are possible for sensor application.
Pressure-induced exotic states in rare earth hexaborides.
Sun, Liling; Wu, Qi
2016-08-01
Finding the exotic phenomena in strongly correlated electron systems (SCESs) and understanding the corresponding microphysics have long been the research frontiers of condensed matter physics. The remarkable examples for the intriguing phenomena discovered in past years include unconventional superconductivity, heavy Fermion behaviors, giant magneto-resistance and so on. A fascinating type of rare earth hexaboride RB6 (R = Sm, Yb, Eu and Ce) belongs to a strongly correlated electron system (SCES), but shows unusual ambient-pressure and high-pressure behaviors beyond the phenomena mentioned above. Particularly, the recent discovery of the coexistence of an unusual metallic surface state and an insulating bulk state in SmB6, known to be a Kondo insulator decades ago, by theoretical calculations and many experimental measurements creates new interest for the investigation of the RB6. This significant progress encourages people to revisit the RB6 with an attempt to establish a new physics that links the SCES and the unusual metallic surface state which is a common feature of a topological insulator (TI). It is well known that pressure has the capability of tuning the electronic structure and modifying the ground state of solids, or even inducing a quantum phase transition which is one of the kernel issues in studies of SCESs. In this brief review, we will describe the progress in high pressure studies on the RB6 based on our knowledge and research interests, mainly focusing on the pressure-induced phenomena in YbB6 and SmB6, especially on the quantum phase transitions and their connections with the valence state of the rare earth ions. Moreover, some related high-pressure results obtained from CeB6 and EuB6 are also included. Finally, a summary is given in the conclusions and perspectives section. PMID:27376406
Pressure-induced exotic states in rare earth hexaborides
NASA Astrophysics Data System (ADS)
Sun, Liling; Wu, Qi
2016-08-01
Finding the exotic phenomena in strongly correlated electron systems (SCESs) and understanding the corresponding microphysics have long been the research frontiers of condensed matter physics. The remarkable examples for the intriguing phenomena discovered in past years include unconventional superconductivity, heavy Fermion behaviors, giant magneto-resistance and so on. A fascinating type of rare earth hexaboride RB6 (R = Sm, Yb, Eu and Ce) belongs to a strongly correlated electron system (SCES), but shows unusual ambient-pressure and high-pressure behaviors beyond the phenomena mentioned above. Particularly, the recent discovery of the coexistence of an unusual metallic surface state and an insulating bulk state in SmB6, known to be a Kondo insulator decades ago, by theoretical calculations and many experimental measurements creates new interest for the investigation of the RB6. This significant progress encourages people to revisit the RB6 with an attempt to establish a new physics that links the SCES and the unusual metallic surface state which is a common feature of a topological insulator (TI). It is well known that pressure has the capability of tuning the electronic structure and modifying the ground state of solids, or even inducing a quantum phase transition which is one of the kernel issues in studies of SCESs. In this brief review, we will describe the progress in high pressure studies on the RB6 based on our knowledge and research interests, mainly focusing on the pressure-induced phenomena in YbB6 and SmB6, especially on the quantum phase transitions and their connections with the valence state of the rare earth ions. Moreover, some related high-pressure results obtained from CeB6 and EuB6 are also included. Finally, a summary is given in the conclusions and perspectives section.
Nuclear magnetization in gallium arsenide quantum dots at zero magnetic field
Sallen, G.; Kunz, S.; Amand, T.; Bouet, L.; Kuroda, T.; Mano, T.; Paget, D.; Krebs, O.; Marie, X.; Sakoda, K.; Urbaszek, B.
2014-01-01
Optical and electrical control of the nuclear spin system allows enhancing the sensitivity of NMR applications and spin-based information storage and processing. Dynamic nuclear polarization in semiconductors is commonly achieved in the presence of a stabilizing external magnetic field. Here we report efficient optical pumping of nuclear spins at zero magnetic field in strain-free GaAs quantum dots. The strong interaction of a single, optically injected electron spin with the nuclear spins acts as a stabilizing, effective magnetic field (Knight field) on the nuclei. We optically tune the Knight field amplitude and direction. In combination with a small transverse magnetic field, we are able to control the longitudinal and transverse components of the nuclear spin polarization in the absence of lattice strain—that is, in dots with strongly reduced static nuclear quadrupole effects, as reproduced by our model calculations. PMID:24500329
Quantum Monte Carlo calculations applied to magnetic molecules
NASA Astrophysics Data System (ADS)
Engelhardt, Larry Paul
In this dissertation, we have implemented a quantum Monte Carlo (QMC) algorithm, and have used it to perform calculations for a variety of finite Heisenberg spin systems. A detailed description of the QMC method has been provided, which is followed by applications of the method to various systems. These applications begin with a detailed analysis of the (calculated) equilibrium magnetization and magnetic susceptibility for a number of Heisenberg Hamiltonians. In particular, we have studied the dependence of these quantities on intrinsic spin s, and have quantified the approach to the classical (s → infinity) limit. These results are not specific to a particular physical system, but are potentially applicable to many systems. We have also analyzed four recently synthesized species of magnetic molecules, each of which is theoretically challenging to the methods that are normally used for such analyses. Using the QMC method, we have distinguished the microscopic (exchange) parameters that describe the interactions in each of these magnetic molecules, and, based upon these parameters, we have made predictions for future experiments. The well-known "negative sign problem" (NSP) can be problematic for QMC calculations. However, for some systems, our analysis was able to proceed despite the NSP. For other systems, this is not the cases, so we have clearly indicated when the NSP is, and is not, insurmountable for these types of calculations.
Ground States of a Disordered Frustrated Quantum Dimer Magnet
NASA Astrophysics Data System (ADS)
Hristov, Alexander; Shapiro, Maxwell; Fisher, Ian; Lee, Minseong; Rodenbach, Linsey; Bernheisel, Ashley; Choi, Eun Sang; Park, Ju-Hyun; Civale, Leonardo; Munsie, Tim; Luke, Graeme
2015-03-01
We present results of thermodynamic measurements of the site-diluted spin-dimer magnet Ba3 (Mn1-xVx)2 O8, including magnetization, torque magnetometry, and AC susceptibility. The parent compound Ba3Mn2O8 is a frustrated S = 1 quantum dimer-magnet with a singlet ground state, and triplet and quintuplet excitations. A magnetic field can be used to tune the energy spectrum of this system, yielding successive triplet and quintuplet condensates at low temperatures. Site substitution with S = 0 V breaks Mn-dimers, introducing site disorder into the high-field ordered states. This substitution also introduces unpaired S = 1 Mn ions, and it has been an open question whether such spins order at low temperatures. Here, we present evidence of the spin-freezing of unpaired Mn ions below 240mK for all compositions measured, from x=0.05 to 0.85. We also present the evolution of the high field ordered state with increasing disorder. NSF DMR-Award 1205165.
Magnetically coupled quantum-flux-latch with wide operation margins
NASA Astrophysics Data System (ADS)
Tsuji, Naoki; Takeuchi, Naoki; Narama, Tatsuya; Ortlepp, Thomas; Yamanashi, Yuki; Yoshikawa, Nobuyuki
2015-11-01
We have been developing adiabatic quantum-flux-parametron (AQFP) circuits as an ultra-low-power superconductor logic for energy-efficient computing. In a previous study, we proposed and demonstrated a quantum-flux-latch (QFL), which is a compact and compatible latch for AQFP logic. The QFL is composed of an AQFP buffer gate and a storage loop, which are directly connected to each other. However, the operation margins were not sufficiently wide due to a trade-off between the operation margins of the storage loop and that of the buffer gate. In this present study, we propose a magnetically coupled QFL (MC-QFL), where the storage loop and the buffer gate are physically separated and magnetically coupled to each other to eliminate the trade-off in the operation margins. The simulation results showed that the critical parameter margin of the MC-QFL is twice as large as that of the previously designed QFL. For comparison, we fabricated and demonstrated both the previously designed QFL and the newly designed MC-QFL. The measurement results showed that the MC-QFL has wider operation margins compared with the previously designed QFL.
Optically Pumped Nuclear Magnetic Resonance in the Quantum Hall Regimes
NASA Astrophysics Data System (ADS)
Barrett, S. E.; Khandelwal, P.; Kuzma, N. N.; Pfeiffer, L. N.; West, K. W.
1997-03-01
Optical pumping enables the direct detection of the nuclear magnetic resonance signal of ^71Ga nuclei located in an electron doped GaAs quantum well.footnote S. E. Barrett et al., Phys. Rev. Lett. 72, 1368 (1994) Using this technique, measurements of the Knight shift (K_S)footnote S. E. Barrett et al., Phys. Rev. Lett. 74, 5112 (1995) and spin-lattice relaxation time (T_1)footnote R. Tycko et al., Science 268, 1460 (1995) have been carried out in the Quantum Hall regimes. This talk will focus on our latest measurements of KS and T1 near Landau level filling ν=1, which extend our earlier results to higher magnetic fields (B=12 Tesla) and lower temperatures (T < 1 Kelvin). We will compare these results to the theoretical predictionsfootnote S. L. Sondhi et al., Phys. Rev. B 47, 16419 (1993); H. A. Fertig et al., Phys. Rev. B 50, 11018 (1994) that the charged excitations of the ν = 1 ground state are novel spin textures called skyrmions. The current status of this picture will be discussed.
Microtesla magnetic resonance imaging with a superconducting quantum interference device
McDermott, Robert; Lee, SeungKyun; ten Haken, Bennie; Trabesinger, Andreas H.; Pines, Alexander; Clarke, John
2004-03-15
We have constructed a magnetic resonance imaging (MRI) scanner based on a dc Superconducting QUantum Interference Device (SQUID) configured as a second-derivative gradiometer. The magnetic field sensitivity of the detector is independent of frequency; it is therefore possible to obtain high-resolution images by prepolarizing the nuclear spins in a field of 300 mT and detecting the signal at 132 fYT, corresponding to a proton Larmor frequency of 5.6 kHz. The reduction in the measurement field by a factor of 10,000 compared with conventional scanners eliminates inhomogeneous broadening of the nuclear magnetic resonance lines, even in fields with relatively poor homogeneity. The narrow linewidths result in enhanced signal-to-noise ratio and spatial resolution for a fixed strength of the magnetic field gradients used to encode the image. We present two-dimensional images of phantoms and pepper slices, obtained in typical magnetic field gradients of 100 fYT/m, with a spatial resolution of about 1mm. We further demonstrate a slice-selected image of an intact pepper. By varying the time delay between removal of the polarizing field and initiation of the spin echo sequence we acquire T1-weighted contrast images of water phantoms, some of which are doped with a paramagnetic salt; here, T1 is the nuclear spin-lattice relaxation time. The techniques presented here could readily be adapted to existing multichannel SQUID systems used for magnetic source imaging of brain signals. Further potential applications include low-cost systems for tumor screening and imaging peripheral regions of the body.
Inelastic neutron scattering studies of novel quantum magnets
NASA Astrophysics Data System (ADS)
Plumb, Kemp W.
Inelastic neutron scattering was used to study the magnetic excitation spectrum of three quantum magnets: (i) the double perovskite Ba2FeReO 6; (ii) the two-dimensional square lattice Heisenberg antiferromagnet Sr2CuO2Cl2; and (iii) the quasi-two-dimensional frustrated two-leg ladder BiCu2PO6. We have conducted inelastic neutron scattering measurements on powder samples of the double perovskite compound Ba2FeReO6. The measurements revealed two well defined dispersing spin wave modes. No excitation gap was observable and the spectrum can be explained with a local moment model incorporating the interactions of Fe spins with spin-orbital locked degrees of freedom on the Re site. The results reveal that both significant electronic correlations and spin-orbit coupling on the Re site play a significant role in the spin dynamics of Ba2FeReO6. High resolution neutron scattering measurements of magnetic excitations in the parent cuprate Sr2CuO2Cl2 reveal a significant dispersion and momentum dependent damping of the zone boundary magnons. We directly compare our measurements with previous resonant inelastic x-ray scattering measurements and find a ~25 meV discrepancy between the two techniques for the measured zone boundary energy at (1/2, 0). The deviations are greatest precisely in the region of phase space where the magnon damping is strongest. This comparison shows that the inelastic x-ray spectrum must contain significant contributions from higher energy excitations not previously considered. Our measurements demonstrate that the high energy continuum of magnetic fluctuations is a ubiquitous feature of the magnetic spectrum among insulating monolayer cuprates, and that these excitations couple to both inelastic neutron and light scattering. A comprehensive series of inelastic neutron scattering measurements was used to investigate spin excitations in the frustrated two-leg ladder compound BiCu2PO6. The measurements revealed six branches of steeply dispersing triplon
Formation of current filaments and magnetic field generation in a quantum current-carrying plasma
Niknam, A. R.; Taghadosi, M. R.; Majedi, S.; Khorashadizadeh, S. M.
2013-09-15
The nonlinear dynamics of filamentation instability and magnetic field in a current-carrying plasma is investigated in the presence of quantum effects using the quantum hydrodynamic model. A new nonlinear partial differential equation is obtained for the spatiotemporal evolution of the magnetic field in the diffusion regime. This equation is solved by applying the Adomian decomposition method, and then the profiles of magnetic field and electron density are plotted. It is shown that the saturation time of filamentation instability increases and, consequently, the instability growth rate and the magnetic field amplitude decrease in the presence of quantum effects.
Quantum Monte Carlo Calculations Applied to Magnetic Molecules
Larry Engelhardt
2006-08-09
We have calculated the equilibrium thermodynamic properties of Heisenberg spin systems using a quantum Monte Carlo (QMC) method. We have used some of these systems as models to describe recently synthesized magnetic molecules, and-upon comparing the results of these calculations with experimental data-have obtained accurate estimates for the basic parameters of these models. We have also performed calculations for other systems that are of more general interest, being relevant both for existing experimental data and for future experiments. Utilizing the concept of importance sampling, these calculations can be carried out in an arbitrarily large quantum Hilbert space, while still avoiding any approximations that would introduce systematic errors. The only errors are statistical in nature, and as such, their magnitudes are accurately estimated during the course of a simulation. Frustrated spin systems present a major challenge to the QMC method, nevertheless, in many instances progress can be made. In this chapter, the field of magnetic molecules is introduced, paying particular attention to the characteristics that distinguish magnetic molecules from other systems that are studied in condensed matter physics. We briefly outline the typical path by which we learn about magnetic molecules, which requires a close relationship between experiments and theoretical calculations. The typical experiments are introduced here, while the theoretical methods are discussed in the next chapter. Each of these theoretical methods has a considerable limitation, also described in Chapter 2, which together serve to motivate the present work. As is shown throughout the later chapters, the present QMC method is often able to provide useful information where other methods fail. In Chapter 3, the use of Monte Carlo methods in statistical physics is reviewed, building up the fundamental ideas that are necessary in order to understand the method that has been used in this work. With these
Quantum critical behavior in heavy electron materials
Yang, Yi-feng; Pines, David
2014-01-01
Quantum critical behavior in heavy electron materials is typically brought about by changes in pressure or magnetic field. In this paper, we develop a simple unified model for the combined influence of pressure and magnetic field on the effectiveness of the hybridization that plays a central role in the two-fluid description of heavy electron emergence. We show that it leads to quantum critical and delocalization lines that accord well with those measured for CeCoIn5, yields a quantitative explanation of the field and pressure-induced changes in antiferromagnetic ordering and quantum critical behavior measured for YbRh2Si2, and provides a valuable framework for describing the role of magnetic fields in bringing about quantum critical behavior in other heavy electron materials. PMID:24912172
Amaral, Jose Jussi; Wan, Jacky; Rodarte, Andrea L.; Ferri, Christopher; Quint, Makiko T.; Pandolfi, Ronald J.; Scheibner, Michael; Hirst, Linda S.; Ghosh, Sayantani
2014-10-22
The design and development of multifunctional composite materials from artificial nano-constituents is one of the most compelling current research areas. This drive to improve over nature and produce ‘meta-materials’ has met with some success, but results have proven limited with regards to both the demonstration of synergistic functionalities and in the ability to manipulate the material properties post-fabrication and in situ. Here, magnetic nanoparticles (MNPs) and semiconducting quantum dots (QDs) are co-assembled in a nematic liquid crystalline (LC) matrix, forming composite structures in which the emission intensity of the quantum dots is systematically and reversibly controlled with a small applied magnetic field (<100 mT). This magnetic field-driven brightening, ranging between a two- to three-fold peak intensity increase, is a truly cooperative effect: the LC phase transition creates the co-assemblies, the clustering of the MNPs produces LC re-orientation at atypical low external field, and this re-arrangement produces compaction of the clusters, resulting in the detection of increased QD emission. These results demonstrate a synergistic, reversible, and an all-optical process to detect magnetic fields and additionally, as the clusters are self-assembled in a fluid medium, they offer the possibility for these sensors to be used in broad ranging fluid-based applications.
Amaral, Jose Jussi; Wan, Jacky; Rodarte, Andrea L; Ferri, Christopher; Quint, Makiko T; Pandolfi, Ronald J; Scheibner, Michael; Hirst, Linda S; Ghosh, Sayantani
2015-01-14
The design and development of multifunctional composite materials from artificial nano-constituents is one of the most compelling current research areas. This drive to improve over nature and produce 'meta-materials' has met with some success, but results have proven limited with regards to both the demonstration of synergistic functionalities and in the ability to manipulate the material properties post-fabrication and in situ. Here, magnetic nanoparticles (MNPs) and semiconducting quantum dots (QDs) are co-assembled in a nematic liquid crystalline (LC) matrix, forming composite structures in which the emission intensity of the quantum dots is systematically and reversibly controlled with a small applied magnetic field (<100 mT). This magnetic field-driven brightening, ranging between a two- to three-fold peak intensity increase, is a truly cooperative effect: the LC phase transition creates the co-assemblies, the clustering of the MNPs produces LC re-orientation at atypical low external field, and this re-arrangement produces compaction of the clusters, resulting in the detection of increased QD emission. These results demonstrate a synergistic, reversible, and an all-optical process to detect magnetic fields and additionally, as the clusters are self-assembled in a fluid medium, they offer the possibility for these sensors to be used in broad ranging fluid-based applications. PMID:25354546
Amaral, Jose Jussi; Wan, Jacky; Rodarte, Andrea L.; Ferri, Christopher; Quint, Makiko T.; Pandolfi, Ronald J.; Scheibner, Michael; Hirst, Linda S.; Ghosh, Sayantani
2014-10-22
The design and development of multifunctional composite materials from artificial nano-constituents is one of the most compelling current research areas. This drive to improve over nature and produce ‘meta-materials’ has met with some success, but results have proven limited with regards to both the demonstration of synergistic functionalities and in the ability to manipulate the material properties post-fabrication and in situ. Here, magnetic nanoparticles (MNPs) and semiconducting quantum dots (QDs) are co-assembled in a nematic liquid crystalline (LC) matrix, forming composite structures in which the emission intensity of the quantum dots is systematically and reversibly controlled with a small appliedmore » magnetic field (<100 mT). This magnetic field-driven brightening, ranging between a two- to three-fold peak intensity increase, is a truly cooperative effect: the LC phase transition creates the co-assemblies, the clustering of the MNPs produces LC re-orientation at atypical low external field, and this re-arrangement produces compaction of the clusters, resulting in the detection of increased QD emission. These results demonstrate a synergistic, reversible, and an all-optical process to detect magnetic fields and additionally, as the clusters are self-assembled in a fluid medium, they offer the possibility for these sensors to be used in broad ranging fluid-based applications.« less
AA-stacked bilayer graphene quantum dots in magnetic field
NASA Astrophysics Data System (ADS)
Belouad, Abdelhadi; Zahidi, Youness; Jellal, Ahmed
2016-05-01
By applying the infinite-mass boundary condition, we analytically calculate the confined states and the corresponding wave functions of AA-stacked bilayer graphene (BLG) quantum dots (QDs) in the presence of an uniform magnetic field B. It is found that the energy spectrum shows two set of levels, which are the double copies of the energy spectrum for single layer graphene, shifted up–down by +γ and -γ , respectively. However, the obtained spectrum exhibits different symmetries between the electron and hole states as well as the intervalley symmetries. It is noticed that, the applied magnetic field breaks all symmetries, except one related to the intervalley electron–hole symmetry, i.e. {E}{{e}}(τ ,m)=-{E}{{h}}(τ ,m). Two different regimes of confinement are found: the first one is due to the infinite-mass barrier at weak B and the second is dominated by the magnetic field as long as B is large. We numerically investigated the basics features of the energy spectrum to show the main similarities and differences with respect to monolayer graphene, AB-stacked BLG and semiconductor QDs. Dedicated to Professor Dr Hachim A Yamani on the occasion of his 70th birthday.
Magnetic reversal dynamics of a quantum system on a picosecond timescale
Kuznetsov, Alexey V; Soloviev, Igor I; Bakurskiy, Sergey V; Tikhonova, Olga V
2015-01-01
Summary We present our approach for a consistent, fully quantum mechanical description of the magnetization reversal process in natural and artificial atomic systems by means of short magnetic pulses. In terms of the simplest model of a two-level system with a magnetic moment, we analyze the possibility of a fast magnetization reversal on the picosecond timescale induced by oscillating or short unipolar magnetic pulses. We demonstrate the possibility of selective magnetization reversal of a superconducting flux qubit using a single flux quantum-based pulse and suggest a promising, rapid Λ-scheme for resonant implementation of this process. In addition, the magnetization reversal treatment is fulfilled within the framework of the macroscopic theory of the magnetic moment, which allows for the comparison and explanation of the quantum and classical behavior. PMID:26665066
Magnetic reversal dynamics of a quantum system on a picosecond timescale.
Klenov, Nikolay V; Kuznetsov, Alexey V; Soloviev, Igor I; Bakurskiy, Sergey V; Tikhonova, Olga V
2015-01-01
We present our approach for a consistent, fully quantum mechanical description of the magnetization reversal process in natural and artificial atomic systems by means of short magnetic pulses. In terms of the simplest model of a two-level system with a magnetic moment, we analyze the possibility of a fast magnetization reversal on the picosecond timescale induced by oscillating or short unipolar magnetic pulses. We demonstrate the possibility of selective magnetization reversal of a superconducting flux qubit using a single flux quantum-based pulse and suggest a promising, rapid Λ-scheme for resonant implementation of this process. In addition, the magnetization reversal treatment is fulfilled within the framework of the macroscopic theory of the magnetic moment, which allows for the comparison and explanation of the quantum and classical behavior. PMID:26665066
Quantum Hall states stabilized in semi-magnetic bilayers of topological insulators.
Yoshimi, R; Yasuda, K; Tsukazaki, A; Takahashi, K S; Nagaosa, N; Kawasaki, M; Tokura, Y
2015-01-01
By breaking the time-reversal symmetry in three-dimensional topological insulators with the introduction of spontaneous magnetization or application of magnetic field, the surface states become gapped, leading to quantum anomalous Hall effect or quantum Hall effect, when the chemical potential locates inside the gap. Further breaking of inversion symmetry is possible by employing magnetic topological insulator heterostructures that host non-degenerate top and bottom surface states. Here we demonstrate the tailored-material approach for the realization of robust quantum Hall states in the bilayer system, in which the cooperative or cancelling combination of the anomalous and ordinary Hall responses from the respective magnetic and non-magnetic layers is exemplified. The appearance of quantum Hall states at filling factor 0 and +1 can be understood by the relationship of energy band diagrams for the two independent surface states. The designable heterostructures of magnetic topological insulator may explore a new arena for intriguing topological transport and functionality. PMID:26497065
Quantum Hall states stabilized in semi-magnetic bilayers of topological insulators
NASA Astrophysics Data System (ADS)
Yoshimi, R.; Yasuda, K.; Tsukazaki, A.; Takahashi, K. S.; Nagaosa, N.; Kawasaki, M.; Tokura, Y.
2015-10-01
By breaking the time-reversal symmetry in three-dimensional topological insulators with the introduction of spontaneous magnetization or application of magnetic field, the surface states become gapped, leading to quantum anomalous Hall effect or quantum Hall effect, when the chemical potential locates inside the gap. Further breaking of inversion symmetry is possible by employing magnetic topological insulator heterostructures that host non-degenerate top and bottom surface states. Here we demonstrate the tailored-material approach for the realization of robust quantum Hall states in the bilayer system, in which the cooperative or cancelling combination of the anomalous and ordinary Hall responses from the respective magnetic and non-magnetic layers is exemplified. The appearance of quantum Hall states at filling factor 0 and +1 can be understood by the relationship of energy band diagrams for the two independent surface states. The designable heterostructures of magnetic topological insulator may explore a new arena for intriguing topological transport and functionality.
Magnetic Microscopy Using a Superconducting Quantum Interference Device
NASA Astrophysics Data System (ADS)
Black, Randall Christopher
1995-01-01
I describe the design, development, and operation of two different scanning probe microscopes which use a dc superconducting quantum interference device (SQUID) as the sensor. Because of the unprecedented magnetic flux sensitivity of the SQUID, these microscopes can image spatial distributions of magnetic fields on a microscopic scale with an exceptional combination of spatial resolution (currently about 10 μm) and static magnetic field sensitivity (about 34 pT Hz^{ -1/2} at 100 Hz). Both microscopes use thin -film high transition-temperature YBa_2Cu _3O_7 SQUIDs. Unlike other SQUID -based techniques which detect weak magnetic fields by coupling a superconducting pickup-coil to the SQUID and using the SQUID as a current amplifier, the scanning SQUID microscopes described here use the loop of the SQUID directly as the sensor, thus achieving the maximum possible spatial resolution, flux sensitivity, and bandwidth. To achieve high spatial resolution, the SQUID must be correspondingly small and close to the surface of the sample being imaged. In the first instrument, the sample is immersed directly in the liquid nitrogen used to cool the SQUID. In the second microscope, a thin sapphire window in a close-spaced dewar allows the imaging of room -temperature samples in air with a spatial resolution as fine as 50 mum. In addition to using the microscope to image static magnetic fields, I developed three other imaging techniques which use the large detection bandwidth of the SQUID. Eddy currents which are induced in metallic samples by an alternating magnetic field can be imaged at frequencies up to about 1 MHz. Using the SQUID as a field rectifier, I am also able to image radio- and microwave-frequency magnetic fields produced by oscillating currents in samples. Finally, by using the oscillating microwave Josephson currents in the SQUID body, I can obtain voltage-tunable microwave eddy-current images of metallic sample up to about 200 GHz. To demonstrate the imaging
Electron spin coherence near room temperature in magnetic quantum dots
Moro, Fabrizio; Turyanska, Lyudmila; Wilman, James; Fielding, Alistair J.; Fay, Michael W.; Granwehr, Josef; Patanè, Amalia
2015-01-01
We report on an example of confined magnetic ions with long spin coherence near room temperature. This was achieved by confining single Mn2+ spins in colloidal semiconductor quantum dots (QDs) and by dispersing the QDs in a proton-spin free matrix. The controlled suppression of Mn–Mn interactions and minimization of Mn–nuclear spin dipolar interactions result in unprecedentedly long phase memory (TM ~ 8 μs) and spin–lattice relaxation (T1 ~ 10 ms) time constants for Mn2+ ions at T = 4.5 K, and in electron spin coherence observable near room temperature (TM ~ 1 μs). PMID:26040432
Quantum Monte Carlo study of magnetism in the Lieb Lattice
NASA Astrophysics Data System (ADS)
Costa, Natanael; Santos, Tiago; Paiva, Thereza; Dos Santos, Raimundo; Scalettar, Richard
The Hubbard model on the `Lieb lattice' provides an important example of how flat band systems may lead to ferromagnetism: at half filling Lieb proved that a ferrimagnetic ground state can be achieved. Since a rigorous proof that long range order does indeed emerge is still lacking, here we report Determinant Quantum Monte Carlo (DQMC) simulations for this model. We found that the spin correlation between nearest neighbors are always antiferromagnetic, and that for small U ferromagnetic long range order does set in in the ground state. However, spatial spin correlations weaken as U is increased, and we established that long range order is suppressed above Uc ~ 4 . 5 . We obtain the dependence of the magnetization with the on-site repulsion U, and show that it displays a maximum at U ~ 3 . The behavior of the compressibility and of the double occupancy across this transition is also discussed. Also at Department of Physics, UC Davis.
Nuclear-magnetic-resonance quantum calculations of the Jones polynomial
Marx, Raimund; Spoerl, Andreas; Pomplun, Nikolas; Schulte-Herbrueggen, Thomas; Glaser, Steffen J.; Fahmy, Amr; Kauffman, Louis; Lomonaco, Samuel; Myers, John M.
2010-03-15
The repertoire of problems theoretically solvable by a quantum computer recently expanded to include the approximate evaluation of knot invariants, specifically the Jones polynomial. The experimental implementation of this evaluation, however, involves many known experimental challenges. Here we present experimental results for a small-scale approximate evaluation of the Jones polynomial by nuclear magnetic resonance (NMR); in addition, we show how to escape from the limitations of NMR approaches that employ pseudopure states. Specifically, we use two spin-1/2 nuclei of natural abundance chloroform and apply a sequence of unitary transforms representing the trefoil knot, the figure-eight knot, and the Borromean rings. After measuring the nuclear spin state of the molecule in each case, we are able to estimate the value of the Jones polynomial for each of the knots.
Quantum magnetic excitations from stripes in copper-oxide superconductors
NASA Astrophysics Data System (ADS)
Tranquada, John
2005-03-01
Recent inelastic neutron scattering studies show that the magnetic excitation spectra of two well-studied families of cuprate superconductors are much more similar than previously believed. In particular, I will present results we have obtained on La2-xBaxCuO4 (LBCO) with x = 0.125 [1,2]. Using very large single crystals grown at Brookhaven, we were able to measure the magnetic excitations up to 200 meV using the MAPS time-of-flight spectrometer at the ISIS spallation source. While the lowest energy excitations are split incommensurately, these disperse inwards towards the antiferromagnetic wave vector with increasing energy, merging at ˜50 meV. At higher energies the excitations disperse outwards again. There is a significant enhancement of the Q-integrated magnetic scattering near ˜50 meV compared to lower energies, suggestive of quantum correlations and distinct from spin-wave predictions. Many features of the spectrum are quite similar to those found in YBa2Cu3O6.6 [3]. One can qualitatively characterize the results with a universal excitation spectrum, together with a material-dependent spin gap in the superconducting state. It is important to note that the LBCO sample exhibits static stripe order [2], as this has significant implications for the origin of the magnetic excitations in superconducting cuprates. *J. M. Tranquada, H. Woo, T. G. Perring, H. Goka, G. D. Gu, G. Xu, M. Fujita, and K. Yamada, Nature 429, 534 (2004). *M. Fujita, H. Goka, K. Yamada, J. M. Tranquada, and L.-P. Regnault, Phys. Rev. B 70, 104517 (2004). *S. M. Hayden, H. A. Mook, P. C. Dai, T. G. Perring, and F. Dogan, Nature 429, 531 (2004).
Proximate Kitaev quantum spin liquid behaviour in a honeycomb magnet
Banerjee, A.; Bridges, C. A.; Yan, J. -Q.; Aczel, A. A.; Li, L.; Stone, M. B.; Granroth, G. E.; Lumsden, M. D.; Yiu, Y.; Knolle, J.; et al
2016-04-04
Quantum spin liquids (QSLs) are topological states of matter exhibiting remarkable properties such as the capacity to protect quantum information from decoherence. While their featureless ground states have precluded their straightforward experimental identification, excited states are more revealing and particularly interesting due to the emergence of fundamentally new excitations such as Majorana Fermions. Ideal probes of these excitations are inelastic neutron scattering experiments. We report these here for a ruthenium-based material α-RuCl3, continuing a major search (so far concentrated on iridium materials inimical to neutron probes) for realizations of the celebrated Kitaev honeycomb topological QSL. Our measurements confirm the requisitemore » strong spin-orbit coupling and low-temperature magnetic order matching predictions proximate to the QSL. We find stacking faults, inherent to the highly 2D nature of the material, resolve an outstanding puzzle. Crucially, dynamical response measurements above interlayer energy scales are naturally accounted for in terms of deconfinement physics expected for QSLs. Comparing these with recent dynamical calculations involving gauge flux excitations and Majorana fermions of the pure Kitaev model, we propose the excitation spectrum of α-RuCl3 as prime candidate for realization of fractionalized Kitaev physics.« less
Proximate Kitaev quantum spin liquid behaviour in a honeycomb magnet.
Banerjee, A; Bridges, C A; Yan, J-Q; Aczel, A A; Li, L; Stone, M B; Granroth, G E; Lumsden, M D; Yiu, Y; Knolle, J; Bhattacharjee, S; Kovrizhin, D L; Moessner, R; Tennant, D A; Mandrus, D G; Nagler, S E
2016-07-01
Quantum spin liquids (QSLs) are topological states of matter exhibiting remarkable properties such as the capacity to protect quantum information from decoherence. Whereas their featureless ground states have precluded their straightforward experimental identification, excited states are more revealing and particularly interesting owing to the emergence of fundamentally new excitations such as Majorana fermions. Ideal probes of these excitations are inelastic neutron scattering experiments. These we report here for a ruthenium-based material, α-RuCl3, continuing a major search (so far concentrated on iridium materials) for realizations of the celebrated Kitaev honeycomb topological QSL. Our measurements confirm the requisite strong spin-orbit coupling and low-temperature magnetic order matching predictions proximate to the QSL. We find stacking faults, inherent to the highly two-dimensional nature of the material, resolve an outstanding puzzle. Crucially, dynamical response measurements above interlayer energy scales are naturally accounted for in terms of deconfinement physics expected for QSLs. Comparing these with recent dynamical calculations involving gauge flux excitations and Majorana fermions of the pure Kitaev model, we propose the excitation spectrum of α-RuCl3 as a prime candidate for fractionalized Kitaev physics. PMID:27043779
Two-dimensional quantum walk under artificial magnetic field
NASA Astrophysics Data System (ADS)
Yalçınkaya, I.; Gedik, Z.
2015-10-01
We introduce the Peierls substitution to a two-dimensional discrete-time quantum walk on a square lattice to examine the spreading dynamics and the coin-position entanglement in the presence of an artificial gauge field. We use the ratio of the magnetic flux through the unit cell to the flux quantum as a control parameter. For a given flux ratio, we obtain faster spreading for a small number of steps and the walker tends to be highly localized around the origin. Moreover, the spreading of the walk can be suppressed and decreased within a limited time interval for specific rational values of flux ratio. When the flux ratio is an irrational number, even for a large number of steps, the spreading exhibits diffusive behavior rather than the well-known ballistic one as in the classical random walk and there is a significant probability of finding the walker at the origin. We also analyze the coin-position entanglement and show that the asymptotic behavior vanishes when the flux ratio is different from zero and the coin-position entanglement become nearly maximal in a periodic manner in a long time range.
Optically Pumped Nuclear Magnetic Resonance in the Quantum Hall Regimes
NASA Astrophysics Data System (ADS)
Barrett, S. E.; Tycko, R.; Dabbagh, G.; Pfeiffer, L. N.; West, K. W.
1996-03-01
Optical pumping enables the direct detection of the nuclear magnetic resonance signal of ^71Ga nuclei located in an electron doped GaAs quantum well.footnote S. E. Barrett et al., Phys. Rev. Lett. 72, 1368 (1994) Using this technique, measurements of the Knight shiftfootnote S. E. Barrett et al., Phys. Rev. Lett. 74, 5112 (1995) and spin-lattice relaxation timefootnote R. Tycko et al., Science 268, 1460 (1995) have been carried out in the Quantum Hall regimes. It is clear from these measurements that probing the electronic spin degree of freedom can lead to new insights about the effect of interactions on the many-body ground state and low-lying excited states of these systems. For example, the Knight shift measurements provided the first experimental support for the recent theoretical predictionsfootnote S. L. Sondhi et al., Phys. Rev. B 47, 16419 (1993); H. A. Fertig et al., Phys. Rev. B 50, 11018 (1994) that the charged excitations of the ν = 1 ground state are novel spin textures called skyrmions. The current status of this picture will be discussed.
Heat capacity and magnetization of CoNb2O6 near quantum critical point
NASA Astrophysics Data System (ADS)
Liang, Tian; Koohpayeh, Seyed; Krizan, Jason; Dutton, Sian; McQueen, Tyrel; Cava, Robert; Phuan Ong, N.
2012-02-01
CoNb2O6 is a quasi-1D quantum magnet in which magnetic Co^2+ ions are ferromagnetically arranged into nearly isolated chains along the c axis with the magnetic moment confined in the ac-plane. By applying transverse magnetic field along b-axis, quantum phase transition from magnetically ordered phase to paramagnetic phase occurs. Evidence for emergent E8 symmetry was recently obtained by neutron scattering near the quantum critical point (QCP) in an applied transverse magnetic field of 5.5 T We will report on experiments to investigate the behavior of the heat capacity and torque magnetization in the vicinity of the QCP and discuss their implications.
Yang, Yifeng; Urbano, Ricardo; Nicholas, Curro; Pines, David
2009-01-01
We report Knight shift experiments on the superconducting heavy electron material CeCoIn{sub 5} that allow one to track with some precision the behavior of the heavy electron Kondo liquid in the superconducting state with results in agreement with BCS theory. An analysis of the {sup 115}In nuclear quadrupole resonance (NQR) spin-lattice relaxation rate T{sub 1}{sup -1} measurements under pressure reveals the presence of 2d magnetic quantum critical fluctuations in the heavy electron component that are a promising candidate for the pairing mechanism in this material. Our results are consistent with an antiferromagnetic quantum critical point (QCP) located at slightly negative pressure in CeCoIn{sub 5} and provide additional evidence for significant similarities between the heavy electron materials and the high T{sub c} cuprates.
Proposed Robust Entanglement-Based Magnetic Field Sensor Beyond the Standard Quantum Limit
NASA Astrophysics Data System (ADS)
Tanaka, Tohru; Knott, Paul; Matsuzaki, Yuichiro; Dooley, Shane; Yamaguchi, Hiroshi; Munro, William J.; Saito, Shiro
2015-10-01
Recently, there have been significant developments in entanglement-based quantum metrology. However, entanglement is fragile against experimental imperfections, and quantum sensing to beat the standard quantum limit in scaling has not yet been achieved in realistic systems. Here, we show that it is possible to overcome such restrictions so that one can sense a magnetic field with an accuracy beyond the standard quantum limit even under the effect of decoherence, by using a realistic entangled state that can be easily created even with current technology. Our scheme could pave the way for the realizations of practical entanglement-based magnetic field sensors.
Magnetic field dependence of a charge-frustrated state in a triangular triple quantum dot
NASA Astrophysics Data System (ADS)
Seo, M.; Chung, Y.
2013-11-01
We studied the magnetic field dependence of a charge-frustrated state formed in a triangular triple quantum dot. Stability diagrams at various magnetic fields were measured by using two-terminal and three-terminal conductance measurement schemes. We found that the frustrated state broke down at an external magnetic field of around 0.1 T. This result is due to the confinement energy shifts in quantum dots under external magnetic fields. A similar breakdown of the frustrated state was observed when the confinement energy of a quantum dot was intentionally shifted by the plunger gate of the dot, which confirm the reason for the breakdown of the frustrated state under on applied magnetic field. Our measured stability diagrams differed depending on the measurement schemes, which could not be explained by the capacitive interaction model based on an independent particle picture. We believe that the discrepancy is related to the closed electron and hole trajectories inside a triple quantum dot.
Illustrating the quantum approach with an Earth magnetic field MRI
NASA Astrophysics Data System (ADS)
Pars Benli, Kami; Dillmann, Baudouin; Louelh, Ryma; Poirier-Quinot, Marie; Darrasse, Luc
2015-05-01
Teaching imaging of magnetic resonance (MR) today is still as challenging as it has always been, because it requires admitting that we cannot express fundamental questions of quantum mechanics with straightforward language or without using extensive theory. Here we allow students to face a real MR setup based on the Earth's magnetic field. We address the applied side of teaching MR using a device that is affordable and that proves to be sufficiently robust, at universities in Orsay, France, and San Sebastian, Spain, in experimental practicals at undergraduate and graduate levels. We specifically present some of the advantages of low field for measuring R2 relaxation rates, reaching a power of separation of 1.5 μmol on Mn(II) ions between two water bottles each of half a liter. Finally we propose key approaches for the lecturers to adopt when they are asked to pass from theoretical knowledge to teachable knowhow. The outcomes are fast calibration and the MR acquisition protocols, demonstrating the reproducibility of energy transfer during the saturation pulses, and the quantitative nature of MR, with water protons and a helium-3 sample.
NASA Astrophysics Data System (ADS)
Szafran, B.; Poniedziałek, M. R.
2010-08-01
We consider electron transport in a quantum wire with a side-coupled quantum ring in a two-dimensional model that accounts for a finite width of the channels. We use the finite difference technique to solve the scattering problem as well as to determine the ring-localized states of the energy continuum. The backscattering probability exhibits Fano peaks for magnetic fields for which a ring-localized states appear at the Fermi level. We find that the width of the Fano resonances changes at high magnetic field. The width is increased (decreased) for resonant states with current circulation that produce the magnetic dipole moment that is parallel (antiparallel) to the external magnetic field. We indicate that the opposite behavior of Fano resonances due to localized states with clockwise and counterclockwise currents results from the magnetic forces which change the strength of their coupling to the channel and modify the lifetime of localized states.
Enhancement of Quantum Efficiency of Organic Light Emitting Devices by Doping Magnetic Nanoparticles
Sun, Chengjun; Wu, Yue; Xu, Zhihua; Hu, Bin; Bai, Jianmin; Wang, Jian-Ping; Shen, Jian
2007-01-01
Magnetic nanoparticles of CoFe are used as dopants to enhance the quantum efficiency of electroluminance in a single layer organic light emitting device (OLED). The enhancement of quantum efficiency increases with both increasing density of CoFe nanoparticles and external magnetic field. For a given OLED with 0.1 wt % doping, the enhancement of the quantum efficiency reaches {approx}27% and {approx}32% without and with a magnetic field, respectively. The origin of these improvements could be attributed to the simultaneous increases of the portion of excitons among total charge carriers and the fraction of singlets among the total excitons
Quantum aspects of a moving magnetic quadrupole moment interacting with an electric field
Fonseca, I. C.; Bakke, K.
2015-06-15
The quantum dynamics of a moving particle with a magnetic quadrupole moment that interacts with electric and magnetic fields is introduced. By dealing with the interaction between an electric field and the magnetic quadrupole moment, it is shown that an analogue of the Coulomb potential can be generated and bound state solutions can be obtained. Besides, the influence of the Coulomb-type potential on the harmonic oscillator is investigated, where bound state solutions to both repulsive and attractive Coulomb-type potentials are achieved and the arising of a quantum effect characterized by the dependence of the harmonic oscillator frequency on the quantum numbers of the system is discussed.
Pressure-induced superconductivity in europium metal
Debessai, M.; Matsuoka, T.; Hamlin, J.J.; Bi, W.; Meng, Y.; Shimizu, K.; Schilling, J.S.
2010-05-24
Of the 52 known elemental superconductors among the 92 naturally occurring elements in the periodic table, fully 22 only become superconducting under sufficiently high pressure. In the rare-earth metals, the strong local magnetic moments originating from the 4f shell suppress superconductivity. For Eu, however, Johansson and Rosengren have suggested that sufficiently high pressures should promote one of its 4f electrons into the conduction band, changing Eu from a strongly magnetic (J=7/2) 4f{sup 7}-state into a weak Van Vleck paramagnetic (J=0) 4f{sup 6}-state, thus opening the door for superconductivity, as in Am (5f{sup 6}). We report that Eu becomes superconducting above 1.8 K for pressures exceeding 80 GPa, T{sub c} increasing linearly with pressure to 142 GPa at the rate +15 mK/GPa. Eu thus becomes the 53rd elemental superconductor in the periodic table. Synchrotron x-ray diffraction studies to 92 GPa at ambient temperature reveal four structural phase transitions.
Sensing the quantum behaviour of magnetic nanoparticles by electron magnetic resonance.
Fittipaldi, M; Mercatelli, R; Sottini, S; Ceci, P; Falvo, E; Gatteschi, D
2016-02-01
We have investigated Magnetic Nanoparticles (MNPs) of spinel type iron oxide (of approximately 8 nm) mineralized in the internal cavity of the bioreactor ferritin nanocage. In particular, we have used Electron Magnetic Resonance, EMR, spectroscopy and taken advantage of the capacity of the protein shells to control the size of the MNPs. EMR measurements in perpendicular and parallel configurations have been recorded at various temperatures. A model based on the giant spin is used to interpret the experimental results. The analysis indicates that the observed quantum behaviour has to be ascribed to the whole MNP and that the thermal population of excited spin states has a strong influence in the EMR behaviour of MNPs. PMID:26750402
Stabilization of the Rayleigh-Taylor instability in quantum magnetized plasmas
Wang, L. F.; Ye, W. H.; He, X. T.; Yang, B. L.
2012-07-15
In this research, stabilization of the Rayleigh-Taylor instability (RTI) due to density gradients, magnetic fields, and quantum effects, in an ideal incompressible plasma, is studied analytically and numerically. A second-order ordinary differential equation (ODE) for the RTI including quantum corrections, with a continuous density profile, in a uniform external magnetic field, is obtained. Analytic expressions of the linear growth rate of the RTI, considering modifications of density gradients, magnetic fields, and quantum effects, are presented. Numerical approaches are performed to solve the second-order ODE. The analytical model proposed here agrees with the numerical calculation. It is found that the density gradients, the magnetic fields, and the quantum effects, respectively, have a stabilizing effect on the RTI (reduce the linear growth of the RTI). The RTI can be completely quenched by the magnetic field stabilization and/or the quantum effect stabilization in proper circumstances leading to a cutoff wavelength. The quantum effect stabilization plays a central role in systems with large Atwood number and small normalized density gradient scale length. The presence of external transverse magnetic fields beside the quantum effects will bring about more stability on the RTI. The stabilization of the linear growth of the RTI, for parameters closely related to inertial confinement fusion and white dwarfs, is discussed. Results could potentially be valuable for the RTI treatment to analyze the mixing in supernovas and other RTI-driven objects.
Magnetic quantum phase diagram of magnetic impurities in two-dimensional disordered electron systems
NASA Astrophysics Data System (ADS)
Lee, Hyun Yong; Kettemann, Stefan
2014-04-01
The quantum phase diagram of disordered electron systems as a function of the concentration of magnetic impurities nm and the local exchange coupling J is studied in the dilute limit. We take into account the Anderson localization of the electrons by a nonperturbative numerical treatment of the disorder potential. The competition between Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction JRKKY and the Kondo effect, as governed by the temperature scale TK, is known to give rise to a rich magnetic quantum phase diagram, the Doniach diagram. Our numerical calculations show that in a disordered system both the Kondo temperature TK and JRKKY as well as their ratio JRKKY/TK is widely distributed. However, we find a sharp cutoff of that distribution, which allows us to define a critical density of magnetic impurities nc below which Kondo screening wins at all sites of the system above a critical coupling Jc, forming the Kondo phase [see Fig. 3(b)]. As disorder is increased, Jc increases and a spin coupled phase is found to grow at the expense of the Kondo phase. From these distribution functions we derive the magnetic susceptibility which show anomalous power-law behavior. In the Kondo phase that power is determined by the wide distribution of the Kondo temperature, while in the spin coupled phase it is governed by the distribution of JRKKY. At low densities and small J
Sharma, Prerana; Chhajlani, R. K.
2014-03-15
The effect of spin induced magnetization and electrical resistivity incorporating the viscosity of the medium is examined on the Jeans instability of quantum magnetoplasma. Formulation of the system is done by using the quantum magnetohydrodynamic model. The analysis of the problem is carried out by normal mode analysis theory. The general dispersion relation is derived from set of perturbed equations to analyse the growth rate and condition of self-gravitational Jeans instability. To discuss the influence of resistivity, magnetization, and viscosity parameters on Jeans instability, the general dispersion relation is reduced for both transverse and longitudinal mode of propagations. In the case of transverse propagation, the gravitating mode is found to be affected by the viscosity, magnetization, resistivity, and magnetic field strength whereas Jeans criterion of instability is modified by the magnetization and quantum parameter. In the longitudinal mode of propagation, the gravitating mode is found to be modified due to the viscosity and quantum correction in which the Jeans condition of instability is influenced only by quantum parameter. The other non-gravitating Alfven mode in this direction is affected by finite electrical resistivity, spin induced magnetization, and viscosity. The numerical study for the growth rate of Jeans instability is carried out for both in the transverse and longitudinal direction of propagation to the magnetic field. The effect of various parameters on the growth rate of Jeans instability in quantum plasma is analysed.
Ground state and excitations of quantum dots with magnetic impurities
NASA Astrophysics Data System (ADS)
Kaul, Ribhu K.; Ullmo, Denis; Zaránd, Gergely; Chandrasekharan, Shailesh; Baranger, Harold U.
2009-07-01
We consider an “impurity” with a spin degree of freedom coupled to a finite reservoir of noninteracting electrons, a system which may be realized by either a true impurity in a metallic nanoparticle or a small quantum dot coupled to a large one. We show how the physics of such a spin impurity is revealed in the many-body spectrum of the entire finite-size system; in particular, the evolution of the spectrum with the strength of the impurity-reservoir coupling reflects the fundamental many-body correlations present. Explicit calculation in the strong- and the weak-coupling limits shows that the spectrum and its evolution are sensitive to the nature of the impurity and the parity of electrons in the reservoir. The effect of the finite-size spectrum on two experimental observables is considered. First, we propose an experimental setup in which the spectrum may be conveniently measured using tunneling spectroscopy. A rate equation calculation of the differential conductance suggests how the many-body spectral features may be observed. Second, the finite-temperature magnetic susceptibility is presented, both the impurity and the local susceptibilities. Extensive quantum Monte Carlo calculations show that the local susceptibility deviates from its bulk scaling form. Nevertheless, for special assumptions about the reservoir—the “clean Kondo box” model—we demonstrate that finite-size scaling is recovered. Explicit numerical evaluations of these scaling functions are given, both for even and odd parities and for the canonical and the grand-canonical ensembles.
Optically Pumped Nuclear Magnetic Resonance in the Quantum Hall Regimes
NASA Astrophysics Data System (ADS)
Barrett, Sean E.
1998-03-01
Optical pumping enables the direct detection of the nuclear magnetic resonance signal of ^71Ga nuclei located in an electron doped GaAs quantum well.footnote S. E. Barrett et al., Phys. Rev. Lett. 72, 1368 (1994) This OPNMR technique was previously used to measure the Knight shift (K_S)footnote S. E. Barrett et al., Phys. Rev. Lett. 74, 5112 (1995) and spin-lattice relaxation time (T_1)footnote R. Tycko et al., Science 268, 1460 (1995) near Landau level filling ν=1, which provided the first experimental support for the theoretical predictionsfootnote S. L. Sondhi et al., Phys. Rev. B 47, 16419 (1993); H. A. Fertig et al., Phys. Rev. B 50, 11018 (1994) that the charged excitations of the ν = 1 ground state are novel spin textures called skyrmions. We have recently demonstrated that OPNMR is possible in fields up to B=12 Tesla, and temperatures down to T= 0.3 K, making it a viable new probe of the Fractional Quantum Hall Regime. In this talk we will present our latest OPNMR measurements near Landau level filling ν=1/3, which include the first direct measurement of the electron spin polarization at ν=1/3. The spin polarization drops as the filling factor is varied away from ν=1/3, indicating that the quasiparticles and quasiholes are not fully spin-polarized. We will also show how the NMR lineshape away from ν=1/3 changes dramatically at low temperatures, which is due to slowing of the electron dynamics, and a reduction in the motional narrowing of the NMR line. The current understanding of these results will be discussed.
NASA Astrophysics Data System (ADS)
Cruz, C.; Soares-Pinto, D. O.; Brandão, P.; dos Santos, A. M.; Reis, M. S.
2016-02-01
The control of quantum correlations in solid-state systems by means of material engineering is a broad avenue to be explored, since it makes possible steps toward the limits of quantum mechanics and the design of novel materials with applications on emerging quantum technologies. In this context, this letter explores the potential of molecular magnets to be prototypes of materials for quantum information technology. More precisely, we engineered a material and from its geometric quantum discord we found significant quantum correlations up to 9540 K (even without entanglement); and, in addition, a pure singlet state occupied up to around 80 K (above liquid nitrogen temperature). These results could only be achieved due to the carboxylate group promoting a metal-to-metal huge magnetic interaction.
NASA Astrophysics Data System (ADS)
Val'kov, V. V.; Shustin, M. S.
2015-11-01
The dispersion equation of a strongly anisotropic one-dimensional magnet catena-[FeII(ClO4)2{FeIII(bpca)2}]ClO4 containing alternating high-spin (HS) ( S = 2) and low-spin (LS) ( S = 1/2) iron ions is obtained by the diagram technique for Hubbard operators. The analysis of this equation yields six branches in the excitation spectrum of this magnet. It is important that the crystal field for ions with spin S = 2 is described by the Hamiltonian of single-ion easy-plane anisotropy, whose orientation is changed by 90° when passing from one HS iron ion to another. The U( N) transformation technique in the atomic representation is applied to diagonalize a single-ion Hamiltonian with a large number of levels. It is shown that the modulation of the orientation of easy magnetization planes leads to a model of a ferrimagnet with easy-axis anisotropy and to the formation of energy spectrum with a large gap. For HS iron ions, a decrease in the mean value of the spin projection due to quantum fluctuations is calculated. The analysis of the specific features of the spectrum of elementary excitations allows one to establish a correspondence to a generalized Ising model for which the magnetic susceptibility is calculated in a wide range of temperatures by the transfer-matrix method. The introduction of a statistical ensemble that takes into account the presence of chains of different lengths and the presence of iron ions with different spins allows one to describe the experimentally observed modification of the magnetic susceptibility of the magnet under optical irradiation.
Val’kov, V. V. Shustin, M. S.
2015-11-15
The dispersion equation of a strongly anisotropic one-dimensional magnet catena-[Fe{sup II}(ClO{sub 4}){sub 2}(Fe{sup III}(bpca){sub 2})]ClO{sub 4} containing alternating high-spin (HS) (S = 2) and low-spin (LS) (S = 1/2) iron ions is obtained by the diagram technique for Hubbard operators. The analysis of this equation yields six branches in the excitation spectrum of this magnet. It is important that the crystal field for ions with spin S = 2 is described by the Hamiltonian of single-ion easy-plane anisotropy, whose orientation is changed by 90° when passing from one HS iron ion to another. The U(N) transformation technique in the atomic representation is applied to diagonalize a single-ion Hamiltonian with a large number of levels. It is shown that the modulation of the orientation of easy magnetization planes leads to a model of a ferrimagnet with easy-axis anisotropy and to the formation of energy spectrum with a large gap. For HS iron ions, a decrease in the mean value of the spin projection due to quantum fluctuations is calculated. The analysis of the specific features of the spectrum of elementary excitations allows one to establish a correspondence to a generalized Ising model for which the magnetic susceptibility is calculated in a wide range of temperatures by the transfer-matrix method. The introduction of a statistical ensemble that takes into account the presence of chains of different lengths and the presence of iron ions with different spins allows one to describe the experimentally observed modification of the magnetic susceptibility of the magnet under optical irradiation.
Short-range quantum magnetism of ultracold fermions in an optical lattice.
Greif, Daniel; Uehlinger, Thomas; Jotzu, Gregor; Tarruell, Leticia; Esslinger, Tilman
2013-06-14
Quantum magnetism originates from the exchange coupling between quantum mechanical spins. Here, we report on the observation of nearest-neighbor magnetic correlations emerging in the many-body state of a thermalized Fermi gas in an optical lattice. The key to obtaining short-range magnetic order is a local redistribution of entropy, which allows temperatures below the exchange energy for a subset of lattice bonds. When loading a repulsively interacting gas into either dimerized or anisotropic simple cubic configurations of a tunable-geometry lattice, we observe an excess of singlets as compared with triplets consisting of two opposite spins. For the anisotropic lattice, the transverse spin correlator reveals antiferromagnetic correlations along one spatial axis. Our work facilitates addressing open problems in quantum magnetism through the use of quantum simulation. PMID:23704375
Plasma wave instability in a quantum field effect transistor with magnetic field effect
Zhang, Li-Ping; Xue, Ju-Kui
2013-08-15
The current-carrying state of a nanometer Field Effect Transistor (FET) may become unstable against the generation of high-frequency plasma waves and lead to generation of terahertz radiation. In this paper, the influences of magnetic field, quantum effects, electron exchange-correlation, and thermal motion of electrons on the instability of the plasma waves in a nanometer FET are reported. We find that, while the electron exchange-correlation suppresses the radiation power, the magnetic field, the quantum effects, and the thermal motion of electrons can enhance the radiation power. The radiation frequency increases with quantum effects and thermal motion of electrons, but decreases with electron exchange-correlation effect. Interestingly, we find that magnetic field can suppress the quantum effects and the thermal motion of electrons and the radiation frequency changes non-monotonely with the magnetic field. These properties could make the nanometer FET advantageous for realization of practical terahertz oscillations.
NASA Astrophysics Data System (ADS)
Gustin, C.; Faniel, S.; Hackens, B.; De Poortere, E. P.; Shayegan, M.; Bayot, V.
2003-04-01
We investigate the transport properties of semiconductor ballistic cavities subject to a parallel magnetic field. Universal conductance fluctuations are observed on two GaAs/AlGaAs quantum well samples with one and two occupied carrier subbands, respectively. Large differences between the two open quantum dots in both the amplitude and frequency distribution of these fluctuations are analyzed in terms of electron orbital motion and magnetic subband depopulation.
Basic Models in the Quantum Theory of Magnetism
NASA Astrophysics Data System (ADS)
Izyumov, Yu. A.
2003-08-01
We regard the Heisenberg model, the Hubbard model, the tJ-model and the sd-model as the basic models of the quantum theory of magnetism in solids. They can describe localized and itinerant magnets and strongly correlated electron systems. This review is devoted to analytical approaches for these models: diagrammatic techniques and the method of generating functional. The diagrammatic techniques are based on a generalization of the Wick theorem for spin and X operators. Peculiarities of such techniques for the basic models appear because the spin and X operators do not commute on a C-value, but their commutator (anticommutator) is an operator itself. The method of generating functional is a generalization of the Kadanoff-Baym approach, developed earlier for usual Fermi systems. The generating functional describes the interaction of a system with fluctuating fields, and different Green's functions can be treated as variational derivatives with respect to these fields. Such approach allows to derive the equation of motion for the Green's functions in each model in terms of functional derivatives. These equations help to find common features in the behavior of the basic models, particularly in finding the multiplicative structure of one-particle Green's functions. Iteration of the equations generates perturbation theory, which is compared with the diagrammatic techniques. Both approaches are applied to the calculation of the quasiparticle spectrum of the models and of collective excitations. A generalized random phase approximation (GRPA) is suggested for calculation of different dynamical susceptibilities. This approximation is developed in both approaches: the diagrammatic technique and the generating functional method.
Quantum pattern recognition with liquid-state nuclear magnetic resonance
NASA Astrophysics Data System (ADS)
Neigovzen, Rodion; Neves, Jorge L.; Sollacher, Rudolf; Glaser, Steffen J.
2009-04-01
A quantum pattern recognition scheme is presented, which combines the idea of a classic Hopfield neural network with adiabatic quantum computation. Both the input and the memorized patterns are represented by means of the problem Hamiltonian. In contrast to classic neural networks, the algorithm can return a quantum superposition of multiple recognized patterns. A proof of principle for the algorithm for two qubits is provided using a liquid-state NMR quantum computer.
Magnetic adatoms as memory bits: A quantum master equation analysis
NASA Astrophysics Data System (ADS)
Karlewski, Christian; Marthaler, Michael; Märkl, Tobias; Balashov, Timofey; Wulfhekel, Wulf; Schön, Gerd
2015-06-01
Due to underlying symmetries, the ground states of magnetic adatoms may be highly stable, which opens perspectives for application as single-atom memory. A specific example is a single holmium atom (with J =8 ) on a platinum (111) surface for which exceptionally long lifetimes were observed in recent scanning tunneling microscopy studies. For control and read-out, the atom must be coupled to electronic contacts. Hence the spin dynamics of the system is governed by a quantum master equation. Our analysis shows that, in general, it cannot be reduced to a classical master equation in the basis of the unperturbed crystal-field Hamiltonian. Rather, depending on parameters and control fields, "environment-induced superselection" principles choose the appropriate set of basis states, which in turn determines the specific relaxation channels and lifetimes. Our simulations suggest that in ideal situations the lifetimes should be even longer than observed in the experiment. We, therefore, investigate the influence of various perturbations. We also study the initialization process of the state of the Ho atom by applied voltage pulses and conclude that fast, high fidelity preparation, on a 100 -ns time scale, should be possible.
Neutron Scattering Study of Low Dimensional Quantum Magnets
NASA Astrophysics Data System (ADS)
Broholm, Collin
1997-03-01
I review three neutron scattering experiments which have uncovered unusual magnetic phenomena in non-metallic low dimensional quantum antiferromagnets. (Work done in collaboration with M. Adams, G. Aeppli, C. Carlile, S.-W. Cheong, D. Davidović), D. C. Dender, J. F. DiTusa, P. R. Hammar, B. Hessen, T. Ito, S. H. Lee, K. Lefmann, K. Oka, T. G. Perring, A. P. Ramirez, Daniel H. Reich, H. Takagi, A. Taylor, and Guangyong Xu. I present evidence that the low temperature short-range ordered spin configuration in the kagomé bi-layer system SrCr_9pGa_12-9pO_19 is composed of small groups of spins whose dipole moments cancel. I report the first observation of field induced incommensurate spin correlations in the uniform spin 1/2 antiferromagnetic chain copper benzoate, and I discuss new results concerning sub-gap excitations in a spin 1 antiferromagnetic chain with impurity bonds, (Y_1-xCa_x)_2BaNiO_5.
NASA Astrophysics Data System (ADS)
Abolfath, Ramin M.; Trojnar, Anna; Roostaei, Bahman; Brabec, Thomas; Hawrylak, Pawel
2013-06-01
Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins. The exciton is described in terms of electron and heavy-hole spins interacting via exchange interaction with magnetic impurity, via hyperfine interaction with a finite number of nuclear spins and via dipole interaction with photons. The time evolution of the exciton, magnetic impurity and nuclear spins is calculated exactly between quantum jumps corresponding to exciton radiative recombination. The collapse of the wavefunction and the refilling of the quantum dot with a new spin-polarized exciton is shown to lead to the build up of magnetization of the magnetic impurity as well as nuclear spin polarization. The competition between electron spin transfer to magnetic impurity and to nuclear spins simultaneous with the creation of dark excitons is elucidated. The technique presented here opens up the possibility of studying optically induced dynamical magnetic and nuclear polarization in complex spin systems.
Quantum beats in the field ionization of Rydberg atoms in the presence of magnetic fields
NASA Astrophysics Data System (ADS)
Gregoric, Vincent C.; Hastings, Hannah; Carroll, Thomas J.; Noel, Michael W.
2016-05-01
By exciting a coherent superposition and varying its phase evolution, quantum beats in the selective field ionization of Rydberg atoms have been observed. Here, we present a study exploring the effect of electric and magnetic fields on quantum beats. Beginning with a single excited state, a coherent superposition is created by a short electric field pulse in the presence of a static magnetic field. The resulting quantum beats are then observed in the field ionization spectrum. Additionally, millimeter-wave spectroscopy is used to probe the state populations in this superposition. This work is supported by the National Science Foundation under Grants No. 1205895 and No. 1205897.
Group velocity of extraordinary waves in superdense magnetized quantum plasma with spin-1/2 effects
Li Chunhua; Ren Haijun; Yang Weihong; Wu Zhengwei; Chu, Paul K.
2012-12-15
Based on the one component plasma model, a new dispersion relation and group velocity of elliptically polarized extraordinary electromagnetic waves in a superdense quantum magnetoplasma are derived. The group velocity of the extraordinary wave is modified due to the quantum forces and magnetization effects within a certain range of wave numbers. It means that the quantum spin-1/2 effects can reduce the transport of energy in such quantum plasma systems. Our work should be of relevance for the dense astrophysical environments and the condensed matter physics.
Aharonov-Anandan quantum phases and Landau quantization associated with a magnetic quadrupole moment
NASA Astrophysics Data System (ADS)
Fonseca, I. C.; Bakke, K.
2015-12-01
The arising of geometric quantum phases in the wave function of a moving particle possessing a magnetic quadrupole moment is investigated. It is shown that an Aharonov-Anandan quantum phase (Aharonov and Anandan, 1987) can be obtained in the quantum dynamics of a moving particle with a magnetic quadrupole moment. In particular, it is obtained as an analogue of the scalar Aharonov-Bohm effect for a neutral particle (Anandan, 1989). Besides, by confining the quantum particle to a hard-wall confining potential, the dependence of the energy levels on the geometric quantum phase is discussed and, as a consequence, persistent currents can arise from this dependence. Finally, an analogue of the Landau quantization is discussed.
Exact scattering matrix of graphs in magnetic field and quantum noise
Caudrelier, Vincent; Mintchev, Mihail; Ragoucy, Eric
2014-08-15
We consider arbitrary quantum wire networks modelled by finite, noncompact, connected quantum graphs in the presence of an external magnetic field. We find a general formula for the total scattering matrix of the network in terms of its local scattering properties and its metric structure. This is applied to a quantum ring with N external edges. Connecting the external edges of the ring to heat reservoirs, we study the quantum transport on the graph in ambient magnetic field. We consider two types of dynamics on the ring: the free Schrödinger and the free massless Dirac equations. For each case, a detailed study of the thermal noise is performed analytically. Interestingly enough, in presence of a magnetic field, the standard linear Johnson-Nyquist law for the low temperature behaviour of the thermal noise becomes nonlinear. The precise regime of validity of this effect is discussed and a typical signature of the underlying dynamics is observed.
Using thermal boundary conditions to engineer the quantum state of a bulk magnet.
Schmidt, M A; Silevitch, D M; Aeppli, G; Rosenbaum, T F
2014-03-11
The degree of contact between a system and the external environment can alter dramatically its proclivity to quantum mechanical modes of relaxation. We show that controlling the thermal coupling of cubic-centimeter-sized crystals of the Ising magnet LiHo(x)Y(1-x)F4 to a heat bath can be used to tune the system between a glassy state dominated by thermal excitations over energy barriers and a state with the hallmarks of a quantum spin liquid. Application of a magnetic field transverse to the Ising axis introduces both random magnetic fields and quantum fluctuations, which can retard and speed the annealing process, respectively, thereby providing a mechanism for continuous tuning between the destination states. The nonlinear response of the system explicitly demonstrates quantum interference between internal and external relaxation pathways. PMID:24567389
Using thermal boundary conditions to engineer the quantum state of a bulk magnet
Schmidt, M. A.; Silevitch, D. M.; Aeppli, G.; Rosenbaum, T. F.
2014-01-01
The degree of contact between a system and the external environment can alter dramatically its proclivity to quantum mechanical modes of relaxation. We show that controlling the thermal coupling of cubic-centimeter–sized crystals of the Ising magnet LiHoxY1-xF4 to a heat bath can be used to tune the system between a glassy state dominated by thermal excitations over energy barriers and a state with the hallmarks of a quantum spin liquid. Application of a magnetic field transverse to the Ising axis introduces both random magnetic fields and quantum fluctuations, which can retard and speed the annealing process, respectively, thereby providing a mechanism for continuous tuning between the destination states. The nonlinear response of the system explicitly demonstrates quantum interference between internal and external relaxation pathways. PMID:24567389
Omidi, Mahboubeh Faizabadi, Edris
2015-03-21
Magnetic susceptibility is investigated in a man-made elliptical quantum ring in the presence of Rashba spin-orbit interactions and the magnetic flux. It is shown that magnetic susceptibility as a function of magnetic flux changes between negative and positive signs periodically. The periodicity of the Aharonov-Bohm oscillations depends on the geometry of the region where magnetic field is applied, the eccentricity, and number of sites in each chain ring (the elliptical ring is composed of chain rings). The magnetic susceptibility sign can be reversed by tuning the Rashba spin-orbit strength as well. Both the magnetic susceptibility strength and sign can be controlled via external spin-orbit interactions, which can be exploited in spintronics and nanoelectronics.
Magnetotransport study of the pressure-induced antiferromagnetic phase in FeSe
NASA Astrophysics Data System (ADS)
Terashima, Taichi; Kikugawa, Naoki; Kasahara, Shigeru; Watashige, Tatsuya; Matsuda, Yuji; Shibauchi, Takasada; Uji, Shinya
2016-05-01
The resistivity ρ and Hall resistivity ρH are measured on FeSe at pressures up to P =28.3 kbar in magnetic fields up to B =14.5 T. The ρ (B ) and ρH(B ) curves are analyzed with multicarrier models to estimate the carrier density and mobility as a function of P and temperature (T ≤110 K). It is shown that the pressure-induced antiferromagnetic transition is accompanied by an abrupt reduction of the carrier density and scattering. This indicates that the electronic structure is reconstructed significantly by the antiferromagnetic order.
Pressure-Induced Metallization of the Mott Insulator MnO
Patterson, J R; Aracne, C M; Jackson, D D; Weir, S T; Malba, V; Baker, P A; Vohra, Y K
2004-01-12
High-pressure electrical conductivity experiments have been performed on the Mott insulator MnO to a maximum pressure of 106 GPa. We observe a steady decrease in resistivity to 90 GPa, followed by a large, rapid decrease by a factor of 10{sup 5} between 90 and 106 GPa. Temperature cycling the sample at 87 and 106 GPa shows insulating and metallic behavior at these pressures, respectively. Our observations provide strong evidence for a pressure-induced Mott insulator-to-metal transition with an accompanying magnetic collapse beginning at 90 GPa.
Pressure-induced disproportionation in CuBr
NASA Astrophysics Data System (ADS)
Skelton, E. F.; Webb, A. W.; Qadri, S. B.; Ingalls, R. G.; Traquada, J. M.
1983-04-01
CuBr has been pressurized to 8.3 GPa in four separate runs. Prima facie evidence of pressure-induced disproportionation of cuprous bromide into cupric bromide has been observed on release of pressure from 7 GPa. Evidence is also seen of a phase change in CuBr2 above 5.5 GPa.
Model for the light-induced magnetization in singly charged quantum dots
NASA Astrophysics Data System (ADS)
Henriques, A. B.; Cordeiro, R. C.; Koenraad, P. M.; Otten, F. W. M.; Bayer, M.
2015-02-01
Magnetization is induced in an ensemble of quantum dots, each charged with a single electron, when it is illuminated with a short circularly polarized light pulse that is resonant with the fundamental energy gap of the quantum dots. In this investigation, a quantum-mechanical model for the light-induced magnetization is presented. The phase of the magnetization precession as a function of the strength of the magnetic field in a Voigt geometry is in excellent agreement with experimental data measured on (In,Ga)As singly charged quantum dot ensembles. It is demonstrated that the precession of the hole in the trion plays a vital role because it determines the amplitude and phase of the magnetization precession. The model could also be easily extended to describe positively charged quantum dots. We also suggest that our theory, combined with measurements of the phase as a function of magnetic field, can be used as a technique to measure the resonant trion lifetime as a function of QD emission energy.
Supersolid phase induced by correlated hopping in spin-1/2 frustrated quantum magnets.
Schmidt, K P; Dorier, J; Läuchli, A M; Mila, F
2008-03-01
We show that correlated hopping of triplets, which is often the dominant source of kinetic energy in dimer-based frustrated quantum magnets, produces a remarkably strong tendency to form supersolid phases in a magnetic field. These phases are characterized by simultaneous modulation and ordering of the longitudinal and transverse magnetization, respectively. Using quantum Monte Carlo and a semiclassical approach for an effective hard-core boson model with nearest-neighbor repulsion on a square lattice, we prove, in particular, that a supersolid phase can exist even if the repulsion is not strong enough to stabilize an insulating phase at half-filling. Experimental implications for frustrated quantum antiferromagnets in a magnetic field at zero and finite temperature are discussed. PMID:18352679
Influence of external magnetic field on dynamics of open quantum systems
Kalandarov, Sh. A.; Kanokov, Z.; Adamian, G. G.; Antonenko, N. V.
2007-03-15
The influence of an external magnetic field on the non-Markovian dynamics of an open two-dimensional quantum system is investigated. The fluctuations of collective coordinate and momentum and transport coefficients are studied for a charged harmonic oscillator linearly coupled to a neutral bosonic heat bath. It is shown that the dissipation of collective energy slows down with increasing strength of the external magnetic field. The role of magnetic field in the diffusion processes is illustrated by several examples.
Karpman-Washimi magnetization with electron-exchange effects in quantum plasmas
Hong, Woo-Pyo; Jamil, M.; Rasheed, A.; Jung, Young-Dae
2015-07-15
The influence of quantum electron-exchange on the Karpman-Washimi ponderomotive magnetization is investigated in quantum plasmas. The ponderomotive magnetization and the total radiation power due to the non-stationary Karpman-Washimi interaction related to the time-varying field intensity are obtained as functions of the de Broglie wave length, Debye length, and electron-exchange parameter. The result shows that the electron-exchange effect enhances the cyclotron frequency due to the ponderomotive interactions in quantum plasmas. It is also shown that the electron-exchange effect on the Karpman-Washimi magnetization increases with increasing wave number. In addition, the Karpman-Washimi magnetization and the total radiation power increase with an increase in the ratio of the Debye length to the de Broglie wave length. In streaming quantum plasmas, it is shown that the electron-exchange effect enhances the ponderomotive magnetization below the resonant wave number and, however, suppresses the ponderomotive magnetization above the resonant wave number. The variation of the Karpman-Washimi magnetization and the radiation power due to the variation of the electron-exchange effect and plasma parameters is also discussed.
Quantum Criticality and Unconventional Order in Magnetic and Dielectric Material
NASA Astrophysics Data System (ADS)
Rowley, S. E.; Smith, R.; Sutherland, M. L.; Alireza, P.; Saxena, S. S.; Lonzarich, G. G.
2012-12-01
We present an overview of unconventional phenomena arising close to ferromagnetic and ferroelectric quantum phase transitions. The applicability and potential breakdown of traditional field theories of quantum criticality and the emergence of a multiplicity of critical fields in particular will be discussed.
Field-induced magnetization jumps and quantum criticality in the 2D J-Q model
NASA Astrophysics Data System (ADS)
Iaizzi, Adam; Sandvik, Anders
The J-Q model is a `designer hamiltonian' formed by adding a four spin `Q' term to the standard antiferromagnetic S = 1 / 2 Heisenberg model. The Q term drives a quantum phase transition to a valence-bond solid (VBS) state: a non-magnetic state with a pattern of local singlets which breaks lattice symmetries. The elementary excitations of the VBS are triplons, i.e. gapped S=1 quasiparticles. There is considerable interest in the quantum phase transition between the Néel and VBS states as an example of deconfined quantum criticality. Near the phase boundary, triplons deconfine into pairs of bosonic spin-1/2 excitations known as spinons. Using exact diagonalization and the stochastic series expansion quantum monte carlo method, we study the 2D J-Q model in the presence of an external magnetic field. We use the field to force a nonzero density of magnetic excitations at T=0 and look for signatures of Bose-Einstein condensation of spinons. At higher magnetic fields, there is a jump in the induced magnetization caused by the onset of an effective attractive interaction between magnons on a ferromagnetic background. We characterize the first order quantum phase transition and determine the minimum value of the coupling ratio q ≡ Q / J required to produce this jump. Funded by NSF DMR-1410126.
Longitudinal wave function control in single quantum dots with an applied magnetic field
Cao, Shuo; Tang, Jing; Gao, Yunan; Sun, Yue; Qiu, Kangsheng; Zhao, Yanhui; He, Min; Shi, Jin-An; Gu, Lin; Williams, David A.; Sheng, Weidong; Jin, Kuijuan; Xu, Xiulai
2015-01-01
Controlling single-particle wave functions in single semiconductor quantum dots is in demand to implement solid-state quantum information processing and spintronics. Normally, particle wave functions can be tuned transversely by an perpendicular magnetic field. We report a longitudinal wave function control in single quantum dots with a magnetic field. For a pure InAs quantum dot with a shape of pyramid or truncated pyramid, the hole wave function always occupies the base because of the less confinement at base, which induces a permanent dipole oriented from base to apex. With applying magnetic field along the base-apex direction, the hole wave function shrinks in the base plane. Because of the linear changing of the confinement for hole wave function from base to apex, the center of effective mass moves up during shrinking process. Due to the uniform confine potential for electrons, the center of effective mass of electrons does not move much, which results in a permanent dipole moment change and an inverted electron-hole alignment along the magnetic field direction. Manipulating the wave function longitudinally not only provides an alternative way to control the charge distribution with magnetic field but also a new method to tune electron-hole interaction in single quantum dots. PMID:25624018
Jeans instability of rotating magnetized quantum plasma: Influence of radiation
Joshi, H.; Pensia, R. K.
2015-07-31
The effect of radiative heat-loss function and rotation on the Jeans instability of quantum plasma is investigated. The basic set of equations for this problem is constructed by considering quantum magnetohydrodynamic (QMHD) model. Using normal mode analysis, the general dispersion relation is obtained. This dispersion relation is studied in both, longitudinal and transverse direction of propagations. In both case of longitudinal and transverse direction of propagation, the Jeans instability criterion is modified due to presence of radiative heat-loss function and quantum correction.
Thermodynamic behaviour of Rashba quantum dot in the presence of magnetic field
NASA Astrophysics Data System (ADS)
Sukirti, Gumber; Manoj, Kumar; Pradip, Kumar Jha; Man, Mohan
2016-05-01
The thermodynamic properties of an InSb quantum dot have been investigated in the presence of Rashba spin–orbit interaction and a static magnetic field. The energy spectrum and wave-functions for the system are obtained by solving the Schrodinger wave-equation analytically. These energy levels are employed to calculate the specific heat, entropy, magnetization and susceptibility of the quantum dot system using canonical formalism. It is observed that the system is susceptible to maximum heat absorption at a particular value of magnetic field which depends on the Rashba coupling parameter as well as the temperature. The variation of specific heat shows a Schottky-like anomaly in the low temperature limit and rapidly converges to the value of 2k B with the further increase in temperature. The entropy of the quantum dot is found to be inversely proportional to the magnetic field but has a direct variation with temperature. The substantial effect of Rashba spin–orbit interaction on the magnetic properties of quantum dot is observed at low values of magnetic field and temperature. Project support by the University Grants Commission, India, the Department of Science and Technology, and the University Grants Commission–Basic Science Research (UGC-BSR).
Magnetic transitions and quantum criticality in the three-dimensional Hubbard model
NASA Astrophysics Data System (ADS)
Schäfer, Thomas; Katanin, Andrey; Held, Karsten; Toschi, Alessandro
We analyze the (quantum) critical properties of the simplest model for electronic correlations, the Hubbard model, in three spatial dimensions by means of the dynamical mean field theory (DMFT, including all local correlations) and the dynamical vertex approximation (D ΓA, including non-local correlations on all length scales). Both in the half-filled/unfrustrated and in the hole-doped system the transition temperature is significantly lowered by including non-local fluctuations.In the latter case, however, the magnetic order becomes incommensurate, eventually leading to a complete suppression of the order and giving rise to a magnetic quantum critical point (QCP) at zero temperature. We analyze the (quantum) critical properties of this QCP (e.g. critical exponents) and relate our findings to the standard theory of quantum criticality in metals, the Hertz-Millis-Moriya theory. Solids4Fun, Austrian Science Fund (FWF, Project ID 1243).
Zeeman mapping of probability densities in square quantum wells using magnetic probes
NASA Astrophysics Data System (ADS)
Prechtl, G.; Heiss, W.; Bonanni, A.; Jantsch, W.; Mackowski, S.; Janik, E.; Karczewski, G.
2000-06-01
We use a method to probe experimentally the probability density of carriers confined in semiconductor quantum structures. The exciton Zeeman splitting in quantum wells containing a single, ultranarrow magnetic layer is studied depending on the layer position. In particular, a system consisting of a 1/4 monolayer MnTe embedded at varying positions in nonmagnetic CdTe/CdMgTe quantum wells is investigated. The sp-d exchange interaction results in a drastic increase of the Zeeman splitting, which, because of the strongly localized nature of this interaction, sensitively depends on the position of the MnTe submonolayer in the quantum well. For various interband transitions we show that the dependence of the exciton Zeeman splitting on the position of the magnetic layer directly maps the probability density of free holesin the growth direction.
Mechanism of pressure-induced gelation of milk.
Keenan, R D; Young, D J; Tier, C M; Jones, A D; Underdown, J
2001-07-01
The pressure-induced gelation of concentrated skimmed milk and milk-sugar mixtures was studied to discover the main components responsible for gelation. The major protein component responsible for gelation is micellar casein. Gelation occurs at similar pressures to casein micelle disintegration in dilute milk, and both can be prevented by inclusion of excess calcium chloride. Transmission electron micrographs show that the protein network is formed from particles with diameters approximately an order of magnitude smaller than those of intact casein micelles. Gelation occurs on decompression and is found to be baroreversible. Concentrations of sugar up to 30% reduce the critical concentration of casein required for gelation, but higher sugar concentrations inhibit gelation. A mechanism of gelation based on the aggregation of casein submicelles formed by pressure-induced disintegration of casein micelles is proposed. Observations on the effect of sucrose on gelation are discussed in terms of the influence of sugars on the solvent quality in aqueous casein systems. PMID:11453781
Thickness Dependence of the Quantum Anomalous Hall Effect in Magnetic Topological Insulator Films.
Feng, Xiao; Feng, Yang; Wang, Jing; Ou, Yunbo; Hao, Zhenqi; Liu, Chang; Zhang, Zuocheng; Zhang, Liguo; Lin, Chaojing; Liao, Jian; Li, Yongqing; Wang, Li-Li; Ji, Shuai-Hua; Chen, Xi; Ma, Xucun; Zhang, Shou-Cheng; Wang, Yayu; He, Ke; Xue, Qi-Kun
2016-08-01
The evolution of the quantum anomalous Hall effect with the thickness of Cr-doped (Bi,Sb)2 Te3 magnetic topological insulator films is studied, revealing how the effect is caused by the interplay of the surface states, band-bending, and ferromagnetic exchange energy. Homogeneity in ferromagnetism is found to be the key to high-temperature quantum anomalous Hall material. PMID:27166762
Magnetic anisotropy in Shiba bound states across a quantum phase transition
NASA Astrophysics Data System (ADS)
Hatter, Nino; Heinrich, Benjamin W.; Ruby, Michael; Pascual, Jose I.; Franke, Katharina J.
2015-11-01
The exchange coupling between magnetic adsorbates and a superconducting substrate leads to Shiba states inside the superconducting energy gap and a Kondo resonance outside the gap. The exchange coupling strength determines whether the quantum many-body ground state is a Kondo singlet or a singlet of the paired superconducting quasiparticles. Here we use scanning tunnelling spectroscopy to identify the different quantum ground states of manganese phthalocyanine on Pb(111). We observe Shiba states, which are split into triplets by magnetocrystalline anisotropy. Their characteristic spectral weight yields an unambiguous proof of the nature of the quantum ground state. Our results provide experimental insights into the phase diagram of a magnetic impurity on a superconducting host and shine light on the effects induced by magnetic anisotropy on many-body interactions.
Magnetic anisotropy in Shiba bound states across a quantum phase transition
Hatter, Nino; Heinrich, Benjamin W.; Ruby, Michael; Pascual, Jose I.; Franke, Katharina J.
2015-01-01
The exchange coupling between magnetic adsorbates and a superconducting substrate leads to Shiba states inside the superconducting energy gap and a Kondo resonance outside the gap. The exchange coupling strength determines whether the quantum many-body ground state is a Kondo singlet or a singlet of the paired superconducting quasiparticles. Here we use scanning tunnelling spectroscopy to identify the different quantum ground states of manganese phthalocyanine on Pb(111). We observe Shiba states, which are split into triplets by magnetocrystalline anisotropy. Their characteristic spectral weight yields an unambiguous proof of the nature of the quantum ground state. Our results provide experimental insights into the phase diagram of a magnetic impurity on a superconducting host and shine light on the effects induced by magnetic anisotropy on many-body interactions. PMID:26603561
Transport through a strongly coupled graphene quantum dot in perpendicular magnetic field
2011-01-01
We present transport measurements on a strongly coupled graphene quantum dot in a perpendicular magnetic field. The device consists of an etched single-layer graphene flake with two narrow constrictions separating a 140 nm diameter island from source and drain graphene contacts. Lateral graphene gates are used to electrostatically tune the device. Measurements of Coulomb resonances, including constriction resonances and Coulomb diamonds prove the functionality of the graphene quantum dot with a charging energy of approximately 4.5 meV. We show the evolution of Coulomb resonances as a function of perpendicular magnetic field, which provides indications of the formation of the graphene specific 0th Landau level. Finally, we demonstrate that the complex pattern superimposing the quantum dot energy spectra is due to the formation of additional localized states with increasing magnetic field. PMID:21711781
Rauf Abdullah, Nzar; Tang, Chi-Shung; Manolescu, Andrei; Gudmundsson, Vidar
2016-09-21
We investigate theoretically the balance of the static magnetic and the dynamical photon forces in the electron transport through a quantum dot in a photon cavity with a single photon mode. The quantum dot system is connected to external leads and the total system is exposed to a static perpendicular magnetic field. We explore the transport characteristics through the system by tuning the ratio, [Formula: see text], between the photon energy, [Formula: see text], and the cyclotron energy, [Formula: see text]. Enhancement in the electron transport with increasing electron-photon coupling is observed when [Formula: see text]. In this case the photon field dominates and stretches the electron charge distribution in the quantum dot, extending it towards the contact area for the leads. Suppression in the electron transport is found when [Formula: see text], as the external magnetic field causes circular confinement of the charge density around the dot. PMID:27420809
NASA Astrophysics Data System (ADS)
Abdelrahman, A.; Vasiliev, M.; Alameh, K.
2011-06-01
We investigate the existence of the macroscopic quantum phase in trapped ultracold quantum degenerate gases in an asymmetrical two-dimensional magnetic lattice. We show the key to adiabatically control the tunneling in the new two-dimensional magnetic lattice by means of external magnetic bias fields. In solving the system of coupled time-dependent differential equations, described here by the Boson Josephson Junctions (BJJs), we used an order parameter that includes both time-dependent variational parameters to describe the fractional population at each lattice site and the phase difference to quantify the macroscopic quantum phase signature. A dynamical oscillation of the fractional population and the phase difference at each individual lattice site is observed when solving the BJJs system.
Finite-temperature Dynamics and Quantum Criticality in a Model for Insulating Magnets
NASA Astrophysics Data System (ADS)
Wu, Jianda; Yang, Wang; Wu, Congjun; Si, Qimiao
Theoretical understanding of the finite-temperature dynamics in quantum critical systems is a challenging problem, due to the mixing of thermal and quantum fluctuations. Recently, neutron scattering experiments in the three-dimensional quantum dimmer material TlCuCl3 under pressure tuning have mapped out the magnetic dynamics at finite temperatures in the quantum critical regime, thereby providing the opportunity for systematic understandings. In this work, we calculate the spin spectral function of an O (n) symmetric field theory using a field-theory procedure to two loops. We calculate the temperature dependence of the energy and damping rate of the spin excitations in the quantum critical regime, demonstrate a good agreement with the experimental results, and determine the parameter regime of the field theory that is appropriate for TlCuCl3. From our calculations we can also suggest further experimental means to test the applicability of the underlying field theory in this and related systems.
Ultrafast high-fidelity initialization of a quantum-dot spin qubit without magnetic fields
NASA Astrophysics Data System (ADS)
Mar, Jonathan D.; Baumberg, Jeremy J.; Xu, Xiulai; Irvine, Andrew C.; Williams, David A.
2014-12-01
We demonstrate the initialization of a single quantum-dot hole spin with high fidelity (lower bound >97 %), on picosecond time scales, and without the need for magnetic fields. Using the initialization scheme based on rapid electric-field ionization of a resonantly excited exciton, this is achieved by employing a self-assembled quantum dot with a low conduction-to-valence band offset ratio, allowing control of the relative electron and hole tunneling rates over three orders of magnitude. This large difference in tunneling rates could permit spin-storage efficiencies >99.5 % by fast-switching to a low electric-field condition. Our results may provide a practical route towards ultrafast high-fidelity initialization of individual quantum-dot hole spins for the implementation of quantum error correction in a scalable spin-based quantum computer.
NASA Astrophysics Data System (ADS)
Gustin, C.; Faniel, S.; Hackens, B.; Melinte, S.; Shayegan, M.; Bayot, V.
2003-12-01
We report on conductance fluctuations of ballistic quantum dots in a strictly parallel magnetic field B. The quantum dots are patterned in two-dimensional electron gases (2DEG’s), confined to 15- and 45-nm-thick GaAs quantum wells (QW) with one and two occupied subbands at B=0, respectively. For both dots we observe universal conductance fluctuations (UCF’s) and, in the case of the wide QW dot, a reduction in their amplitude at large B. Our data suggest that the finite thickness of the 2DEG and the orbital effect are responsible for the parallel B-induced UCF’s.
Magnetic and superconducting quantum critical behavior of itinerant electronic systems
NASA Astrophysics Data System (ADS)
Sknepnek, Rastko
Quantum phase transitions occur at zero temperature as a function of some non-thermal parameter, e.g., pressure or chemical composition. In addition to being of fundamental interest, quantum phase transitions are important because they are believed to underlie a number of interesting low temperature phenomena. Quantum phase transitions differ from the classical phase transitions in many important aspects, two of them being (i) the mode-coupling effects and (ii) the behavior in the presence of disorder. We devote two projects of this dissertation to each of the two. First, we investigate the quantum phase transition of itinerant electrons from a paramagnet to a state which displays long-period helical structures due to a Dzyaloshinskii instability of the ferromagnetic state. In particular, we study how the self generated effective long-range interaction recently identified in itinerant quantum ferromagnets is cut-off by the helical ordering. Second, we discuss a quantum phase transition between a disordered metal and an exotic (non-s-wave) superconductor. Like in the case of ferromagnetic quantum phase transition mode coupling effects lead to an effective long-range interaction between the anomalous density fluctuations. We find that the asymptotic critical region is characterized by run-away flow to large disorder. However, for weak coupling, this region is very narrow, and it is preempted by a wide crossover regime with mean-field critical behavior. Then, we present results of large-scale Monte Carlo simulations for a 3d Ising model with short range interactions and planar defects. We show that the phase transition in this system is smeared, i.e., there is no single critical temperature, but different parts of the system order at different temperatures. Our Monte-Carlo results are in good agreement with a recent theory. Finally, we present large-scale Monte-Carlo simulations of a 2d bilayer quantum Heisenberg antiferromagnet with random dimer dilution. In contrast
Double-donor complex in vertically coupled quantum dots in a threading magnetic field.
Manjarres-García, Ramón; Escorcia-Salas, Gene Elizabeth; Manjarres-Torres, Javier; Mikhailov, Ilia D; Sierra-Ortega, José
2012-01-01
We consider a model of hydrogen-like artificial molecule formed by two vertically coupled quantum dots in the shape of axially symmetrical thin layers with on-axis single donor impurity in each of them and with the magnetic field directed along the symmetry axis. We present numerical results for energies of some low-lying levels as functions of the magnetic field applied along the symmetry axis for different quantum dot heights, radii, and separations between them. The evolution of the Aharonov-Bohm oscillations of the energy levels with the increase of the separation between dots is analyzed. PMID:23013550
Tomimatsu, Toru Shirai, Shota; Hashimoto, Katsushi Sato, Ken; Hirayama, Yoshiro
2015-08-15
Electric-field-induced nuclear resonance (NER: nuclear electric resonance) involving quantum Hall states (QHSs) was studied at various filling factors by exploiting changes in nuclear spins polarized at quantum Hall breakdown. Distinct from the magnetic dipole interaction in nuclear magnetic resonance, the interaction of the electric-field gradient with the electric quadrupole moment plays the dominant role in the NER mechanism. The magnitude of the NER signal strongly depends on whether electronic states are localized or extended. This indicates that NER is sensitive to the screening capability of the electric field associated with QHSs.
Field-induced magnetic instability and quantum criticality in the antiferromagnet CeCu2Ge2
Liu, Yi; Xie, Donghua; Wang, Xiaoying; Zhu, Kangwei; Yang, Ruilong
2016-01-01
The magnetic quantum criticality in strongly correlated electron systems has been considered to be closely related with the occurrence of unconventional superconductivity. Control parameters such as magnetic field, pressure or chemical doping are frequently used to externally tune the quantum phase transition for a deeper understanding. Here we report the research of a field-induced quantum phase transition using conventional bulk physical property measurements in the archetypal antiferromagnet CeCu2Ge2, which becomes superconductive under a pressure of about 10 GPa with Tc ~ 0.64 K. We offer strong evidence that short-range dynamic correlations start appearing above a magnetic field of about 5 T. Our demonstrations of the magnetic instability and the field-induced quantum phase transition are crucial for the quantum criticality, which may open a new route in experimental investigations of the quantum phase transition in heavy-fermion systems. PMID:26758347
Field-induced magnetic instability and quantum criticality in the antiferromagnet CeCu2Ge2.
Liu, Yi; Xie, Donghua; Wang, Xiaoying; Zhu, Kangwei; Yang, Ruilong
2016-01-01
The magnetic quantum criticality in strongly correlated electron systems has been considered to be closely related with the occurrence of unconventional superconductivity. Control parameters such as magnetic field, pressure or chemical doping are frequently used to externally tune the quantum phase transition for a deeper understanding. Here we report the research of a field-induced quantum phase transition using conventional bulk physical property measurements in the archetypal antiferromagnet CeCu2Ge2, which becomes superconductive under a pressure of about 10 GPa with Tc ~ 0.64 K. We offer strong evidence that short-range dynamic correlations start appearing above a magnetic field of about 5 T. Our demonstrations of the magnetic instability and the field-induced quantum phase transition are crucial for the quantum criticality, which may open a new route in experimental investigations of the quantum phase transition in heavy-fermion systems. PMID:26758347
Field-induced magnetic instability and quantum criticality in the antiferromagnet CeCu2Ge2
NASA Astrophysics Data System (ADS)
Liu, Yi; Xie, Donghua; Wang, Xiaoying; Zhu, Kangwei; Yang, Ruilong
2016-01-01
The magnetic quantum criticality in strongly correlated electron systems has been considered to be closely related with the occurrence of unconventional superconductivity. Control parameters such as magnetic field, pressure or chemical doping are frequently used to externally tune the quantum phase transition for a deeper understanding. Here we report the research of a field-induced quantum phase transition using conventional bulk physical property measurements in the archetypal antiferromagnet CeCu2Ge2, which becomes superconductive under a pressure of about 10 GPa with Tc ~ 0.64 K. We offer strong evidence that short-range dynamic correlations start appearing above a magnetic field of about 5 T. Our demonstrations of the magnetic instability and the field-induced quantum phase transition are crucial for the quantum criticality, which may open a new route in experimental investigations of the quantum phase transition in heavy-fermion systems.
Solving quantum ground-state problems with nuclear magnetic resonance.
Li, Zhaokai; Yung, Man-Hong; Chen, Hongwei; Lu, Dawei; Whitfield, James D; Peng, Xinhua; Aspuru-Guzik, Alán; Du, Jiangfeng
2011-01-01
Quantum ground-state problems are computationally hard problems for general many-body Hamiltonians; there is no classical or quantum algorithm known to be able to solve them efficiently. Nevertheless, if a trial wavefunction approximating the ground state is available, as often happens for many problems in physics and chemistry, a quantum computer could employ this trial wavefunction to project the ground state by means of the phase estimation algorithm (PEA). We performed an experimental realization of this idea by implementing a variational-wavefunction approach to solve the ground-state problem of the Heisenberg spin model with an NMR quantum simulator. Our iterative phase estimation procedure yields a high accuracy for the eigenenergies (to the 10⁻⁵ decimal digit). The ground-state fidelity was distilled to be more than 80%, and the singlet-to-triplet switching near the critical field is reliably captured. This result shows that quantum simulators can better leverage classical trial wave functions than classical computers. PMID:22355607
Excitonic spin-splitting in quantum wells with a tilted magnetic field
NASA Astrophysics Data System (ADS)
Fernandes dos Santos, L.; Castelano, L. K.; Padilha, J. X.; Pusep, Y.; Marques, G. E.; Smirnov, D.; Bakarov, A. K.; Toropov, A. I.; Lopez-Richard, V.
2016-02-01
This work aims to investigate the effects of magnetic field strength and direction on the electronic properties and optical response of GaAs/AlGaAs-based heterostructures. An investigation of the excitonic spin-splitting of a disordered multiple quantum well embedded in a wide parabolic quantum well is presented. The results for polarization-resolved photoluminescence show that the magnetic field dependencies of the excitonic spin-splitting and photoluminescence linewidth are crucially sensitive to magnetic field orientation. Our experimental results are in good agreement with the calculated Zeeman splitting obtained by the Luttinger model, which predicts a hybridization of the spin character of states in the valence band under tilted magnetic fields.
Riva, C.; Peeters, F. M.; Varga, K.
2001-03-15
We present a variational calculation of the spin-singlet and spin-triplet states of a negatively charged exciton (trion) confined to a single quantum well in the presence of a perpendicular magnetic field. We calculated the probability density and the pair correlation function of the singlet and triplet trion states. The dependence of the energy levels and of the binding energy on the well width and on the magnetic field strength was investigated. We compared our results with the available experimental data on GaAs/AlGaAs quantum wells and find that in the low-magnetic-field region (B<18 T) the observed transitions are those of the singlet and the dark triplet trion (with angular momentum L{sub z}=-1), while for high magnetic fields (B>25 T) the dark trion becomes optically inactive and possibly a transition to a bright triplet trion (angular momentum L{sub z}=0) state is observed.
NASA Astrophysics Data System (ADS)
Dzebisashvili, D. M.; Khudaiberdyev, A. A.
2016-06-01
The specific features of quantum oscillations of the magnetization in quasi-two-dimensional wide-band-gap antiferromagnetic semimetals with a low concentration of charge carriers have been considered theoretically. It has been shown that, in these systems, the Fermi energy determined from the analysis of the frequency of the de Haas-van Alphen oscillations according to the standard procedure can differ significantly from the true value. For the correct determination of the Fermi energy in the canted phase, it has been proposed to analyze quantum oscillations of the magnetization M not as a function of the inverse magnetic field 1/ H, but as a function of 1/cosγ, where the angle γ characterizes the inclination angle of the magnetic field with respect to the plane of the quasi-two-dimensional semimetal.
Finite-momentum condensate of magnetic excitons in a bilayer quantum Hall system
NASA Astrophysics Data System (ADS)
Doretto, R. L.; Morais Smith, C.; Caldeira, A. O.
2012-07-01
We study the bilayer quantum Hall system at total filling factor νT=1 within a bosonization formalism which allows us to approximately treat the magnetic exciton as a boson. We show that in the region where the distance between the two layers is comparable to the magnetic length, the ground state of the system can be seen as a finite-momentum condensate of magnetic excitons provided that the excitation spectrum is gapped. We analyze the stability of such a phase within the Bogoliubov approximation first assuming that only one momentum Q is macroscopically occupied and later we consider the same situation for two modes ±Q. We find strong evidences that a first-order quantum phase transition at small interlayer separation takes place from a zero-momentum condensate phase, which corresponds to Halperin 111 state, to a finite-momentum condensate of magnetic excitons.
Jahan K, Luhluh Boda, Aalu; Chatterjee, Ashok
2015-05-15
The problem of an exciton trapped in a three dimensional Gaussian quantum dot is studied in the presence of an external magnetic field. A variational method is employed to obtain the ground state energy of the exciton as a function of the quantum dot size, the confinement strength and the magnetic field. It is also shown that the variation of the size of the exciton with the radius of the quantum dot.
Measurement of radiation-pressure-induced optomechanical dynamics in a suspended Fabry-Perot cavity
Corbitt, Thomas; Ottaway, David; Innerhofer, Edith; Pelc, Jason; Mavalvala, Nergis
2006-08-15
We report on experimental observation of radiation-pressure induced effects in a high-power optical cavity. These effects play an important role in next-generation gravitational wave detectors, as well as in quantum nondemolition interferometers. We measure the properties of an optical spring, created by coupling of an intense laser field to the pendulum mode of a suspended mirror, and also the parametric instability (PI) that arises from the coupling between acoustic modes of the cavity mirrors and the cavity optical mode. We measure an unprecedented optical rigidity of K=(3.08{+-}0.09)x10{sup 4} N/m, corresponding to an optical rigidity that is 6000 times stiffer than the mechanical stiffness, and PI strength R{approx_equal}3. We measure the unstable nature of the optical spring resonance, and demonstrate that the PI can be stabilized by feedback to the frequency of the laser source.
Intrinsic high magnetism in SnO{sub 2} quantum dots
Venkataramana, Bonu Das, A. Dhara, S.; Tyagi, A. K.; Sardar, Manas
2014-04-24
High magnetic moment was observed in SnO{sub 2} quantum dots (QDs) which were prepared by a soft chemical method. SnO{sub 2} QDs were characterized for morphological, structural and optical properties using high resolution tunneling electron microscopy and photoluminescence (PL) spectroscopy, respectively. Magnetism occurred in QDs SnO{sub 2} due to dominant oxygen defects, were studied using PL measurements.
NASA Astrophysics Data System (ADS)
Zhu, Zhenni; Wu, Zhengwei; Li, Chunhua; Yang, Weihong
2014-11-01
A model for the nonlinear properties of obliquely propagating electron acoustic solitary waves in a two-electron populated relativistically quantum magnetized plasma is presented. By using the standard reductive perturbation technique, the Zakharov-Kuznetsov (ZK) equation is derived and this equation gives the solitary wave solution. It is observed that the relativistic effects, the ratio of the cold to hot electron unperturbed number density and the magnetic field normalized by electron cyclotron frequency significantly influence the solitary structures.
Wave packet revivals in a graphene quantum dot in a perpendicular magnetic field
Torres, J. J.
2010-10-15
We study the time evolution of localized wave packets in graphene quantum dots in a perpendicular magnetic field, focusing on the quasiclassical and revival periodicities, for different values of the magnetic field intensities in a theoretical framework. We have considered contributions of the two inequivalent points in the Brillouin zone. The revival time has been found as an observable that shows the break valley degeneracy.
Quantum rings of non-uniform thickness in magnetic field
Rodríguez-Prada, F. A.; García, L. F.; Mikhailov, I. D.
2014-05-15
We consider a model of crater-shaped quantum dot in form of a thin layer whose thickness linearly increases with the distance from the axis. We show that one-particle wave equation for the electron confined in such structure can be completely separated in the adiabatic limit when the quantum dot thickness is much smaller than its lateral dimension. Analytical solutions found for this model has been used as base functions for analysing the effect of non-homogeneity on the electronic spectrum in the framework of the exact diagonalization method.
Individual Mammalian Cell Magnetic Measurements with a Superconducting Quantum Interference Device
NASA Astrophysics Data System (ADS)
Palmstrom, Johanna C.; Brewer, Kimberly; Tee, Sui Seng; Theis, Eric; Rutt, Brian; Moler, Kathryn A.
2015-03-01
Magnetism can be introduced into otherwise nonmagnetic cells by the uptake of superparamagnetic iron oxide (SPIO) nanoparticles. SPIO nanoparticles are used in numerous biomedical applications including cellular therapies and targeted drug delivery. Currently there are few tools capable of characterizing individual magnetic nanoparticles and the magnetic properties of individual mammalian cells loaded with SPIO. Our scanning superconducting quantum interference devices (SQUIDs) are good candidates for these measurements due to their high sensitivity to magnetic dipole moments (approx. 200 μb/ √Hz) In this study, we use a scanning SQUID to image the magnetic flux from SPIO loaded H1299 lung cancer cells. We find that the magnetic moment spatially varies inside the cell with each cell having a unique distribution of moments. We also correlate these magnetic images with optical and scanning electron microscope images. These results show that the SQUID is a useful tool for imaging biological magnetism. The visualization of single cell magnetism and the quantification of magnetic dipole moments in magnetically labeled cells can be used to optimize conventional biological magnetic imaging techniques, such as MRI.
Quantum Anomalous Hall Effect in Low-buckled Honeycomb Lattice with In-plane Magnetization
NASA Astrophysics Data System (ADS)
Ren, Yafei; Pan, Hui; Yang, Fei; Li, Xin; Qiao, Zhenhua; Zhenhua Qiao's group Team; Hui Pan's group Team
With out-of-plane magnetization, the quantum anomalous Hall effect has been extensively studied in quantum wells and two-dimensional atomic crystal layers. Here, we investigate the possibility of realizing quantum anomalous Hall effect (QAHE) in honeycomb lattices with in-plane magnetization. We show that the QAHE can only occur in low-buckled honeycomb lattice where both intrinsic and intrinsic Rashba spin-orbit coupling appear spontaneously. The extrinsic Rashba spin-orbit coupling is detrimental to this phase. In contrast to the out-of-plane magnetization induced QAHE, the QAHE from in-plane magnetization is achieved in the vicinity of the time reversal symmetric momenta at M points rather than Dirac points. In monolayer case, the QAHE can be characterized by Chern number = +/- 1 whereas additional phases with Chern number = +/- 2 appear in chiral stacked bilayer system. The Chern number strongly depends on the orientation of the magnetization. The bilayer system also provides additional tunability via out-of-plane electric field, which can reduce the critical magnetization strength required to induce QAHE. It can also lead to topological phase transitions from = +/- 2 to +/- 1 and finally to 0 Equal contribution from Yafei Ren and Hui Pan.
Evidence for magnetic clusters in Ni1-xVx close to the quantum critical concentration
NASA Astrophysics Data System (ADS)
Wang, R.; Ubaid-Kassis, S.; Schroeder, A.; Baker, P. J.; Pratt, F. L.; Blundell, S. J.; Lancaster, T.; Franke, I.; Möller, J. S.; Vojta, T.
2015-03-01
The d-metal alloy Ni1-xVx undergoes a quantum phase transition from a ferromagnetic ground state to a paramagnetic ground state as the vanadium concentration x is increased. We present magnetization, ac-susceptibility and muon-spin relaxation data at several vanadium concentrations near the critical concentration xc ~ 11.6 % at which the onset of ferromagnetic order is suppressed to zero temperature. Below xc, the muon data reveal a broad magnetic field distribution indicative of a long-range ordered ferromagnetic state with spatial disorder. We show evidence of magnetic clusters in the ferromagnetic phase and close to the phase boundary in this disordered itinerant system as an important generic ingredient of a disordered quantum phase transition. In contrast, the temperature dependence of the magnetic susceptibility above xc is best described in terms of a magnetic quantum Griffiths phase with a power-law distribution of fluctuation rates of dynamic magnetic clusters. At the lowest temperatures, the onset of a short-range ordered cluster-glass phase is recognized by an increase in the muon depolarization in transverse fields and maxima in ac-susceptibility.
Time-resolved magnetophotoluminescence studies of magnetic polaron dynamics in type-II quantum dots
NASA Astrophysics Data System (ADS)
Barman, B.; Oszwałdowski, R.; Schweidenback, L.; Russ, A. H.; Pientka, J. M.; Tsai, Y.; Chou, W.-C.; Fan, W. C.; Murphy, J. R.; Cartwright, A. N.; Sellers, I. R.; Petukhov, A. G.; Žutić, I.; McCombe, B. D.; Petrou, A.
2015-07-01
We used continuous wave photoluminescence (cw-PL) and time-resolved photoluminescence (TR-PL) spectroscopy to compare the properties of magnetic polarons (MP) in two related spatially indirect II-VI epitaxially grown quantum dot systems. In the ZnTe /(Zn ,Mn )Se system the holes are confined in the nonmagnetic ZnTe quantum dots (QDs), and the electrons reside in the magnetic (Zn,Mn)Se matrix. On the other hand, in the (Zn ,Mn )Te /ZnSe system, the holes are confined in the magnetic (Zn,Mn)Te QDs, while the electrons remain in the surrounding nonmagnetic ZnSe matrix. The magnetic polaron formation energies EMP in both systems were measured from the temporal redshift of the band-edge emission. The magnetic polaron exhibits distinct characteristics depending on the location of the Mn ions. In the ZnTe /(Zn ,Mn )Se system the magnetic polaron shows conventional behavior with EMP decreasing with increasing temperature T and increasing magnetic field B . In contrast, EMP in the (Zn ,Mn )Te /ZnSe system has unconventional dependence on temperature T and magnetic field B ; EMP is weakly dependent on T as well as on B . We discuss a possible origin for such a striking difference in the MP properties in two closely related QD systems.
Giant magnetic anisotropy and quantum tunneling of the magnetization in Li2(Li1-xFex)N
NASA Astrophysics Data System (ADS)
Jesche, Anton; McCallum, R. William; Thimmaiah, Srinivasa; Jacobs, Jenee L.; Taufour, Valentin; Kreyssig, Andreas; Houk, Robert S.; Bud'Ko, Sergey L.; Canfield, Paul C.
2014-03-01
The magnetic anisotropy of 3 d transition metals is usually considered to be weak, mainly due to the widely known paradigm of orbital quenching. However, a rare interplay of crystal electric field effects and spin-orbit coupling causes a large orbital contribution to the magnetic moment of iron in Li2(Li1-xFex)N. This leads, not only to large magnetic moments of ~ 5 μB per iron atom but, also, to an enormous magnetic anisotropy field that extrapolates to more than 200 Tesla. Magnetic hysteresis emerges for T <= 50 K and the coercivity fields of more than 11 Tesla exceed even the hardest 4 f electron based ferromagnets. Li2(Li1-xFex)N not only has a clear and remarkable anisotropy, generally not associated with iron moments, but also shows time-dependence more consistent with molecular magnets. In particular for low iron concentrations x << 1 the spin-inversion is dominated by a macroscopic tunneling process rather than by thermal excitations. It is shown that the huge magnetic anisotropy makes Li2(Li1-xFex)N (i) an ideal model system to study macroscopic quantum effects at elevated temperatures and (ii) a basis for novel magnetic functional materials. This work is supported by the US DOE, Basic Energy Sciences under Contract No. DE-AC02-07CH11358.
Ghosh, Sayandip; Raghuvanshi, Nimisha; Mohapatra, Shubhajyoti; Kumar, Ashish; Singh, Avinash
2016-09-14
Effective spin couplings and spin fluctuation induced quantum corrections to sublattice magnetization are obtained in the [Formula: see text] AF state of a realistic three-orbital interacting electron model involving xz, yz and xy Fe 3d orbitals, providing insight into the multi-orbital quantum antiferromagnetism in iron pnictides. The xy orbital is found to be mainly responsible for the generation of strong ferromagnetic spin coupling in the b direction, which is critically important to fully account for the spin wave dispersion as measured in inelastic neutron scattering experiments. The ferromagnetic spin coupling is strongly suppressed as the xy band approaches half filling, and is ascribed to particle-hole exchange in the partially filled xy band. The strongest AF spin coupling in the a direction is found to be in the orbital off-diagonal sector involving the xz and xy orbitals. First order quantum corrections to sublattice magnetization are evaluated for the three orbitals, and yield a significant [Formula: see text] average reduction from the Hartree-Fock value. PMID:27406889
NASA Astrophysics Data System (ADS)
Ghosh, Sayandip; Raghuvanshi, Nimisha; Mohapatra, Shubhajyoti; Kumar, Ashish; Singh, Avinash
2016-09-01
Effective spin couplings and spin fluctuation induced quantum corrections to sublattice magnetization are obtained in the (π,0) AF state of a realistic three-orbital interacting electron model involving xz, yz and xy Fe 3d orbitals, providing insight into the multi-orbital quantum antiferromagnetism in iron pnictides. The xy orbital is found to be mainly responsible for the generation of strong ferromagnetic spin coupling in the b direction, which is critically important to fully account for the spin wave dispersion as measured in inelastic neutron scattering experiments. The ferromagnetic spin coupling is strongly suppressed as the xy band approaches half filling, and is ascribed to particle-hole exchange in the partially filled xy band. The strongest AF spin coupling in the a direction is found to be in the orbital off-diagonal sector involving the xz and xy orbitals. First order quantum corrections to sublattice magnetization are evaluated for the three orbitals, and yield a significant 37% average reduction from the Hartree–Fock value.
Bose-Einstein Condensation and Bose Glasses in an S = 1 Organo-metallic quantum magnet
Zapf, Vivien
2012-06-01
I will speak about Bose-Einstein condensation (BEC) in quantum magnets, in particular the compound NiCl2-4SC(NH2)2. Here a magnetic field-induced quantum phase transition to XY antiferromagnetism can be mapped onto BEC of the spins. The tuning parameter for BEC transition is the magnetic field rather than the temperature. Some interesting phenomena arise, for example the fact that the mass of the bosons that condense can be strongly renormalized by quantum fluctuations. I will discuss the utility of this mapping for both understanding the nature of the quantum magnetism and testing the thermodynamic limit of Bose-Einstein Condensation. Furthermore we can dope the system in a clean and controlled way to create the long sought-after Bose Glass transition, which is the bosonic analogy of Anderson localization. I will present experiments and simulations showing evidence for a new scaling exponent, which finally makes contact between theory and experiments. Thus we take a small step towards the difficult problem of understanding the effect of disorder on bosonic wave functions.
Inverse parabolic quantum dot: The transition energy under magnetic field effect
NASA Astrophysics Data System (ADS)
Safwan, S. A.; El Meshed, Nagwa
2016-08-01
We present here, the evolution of the transition energy with a static magnetic field, when the electron and the hole are confined in inverse parabolic quantum dot (IPQD). The unexpected behavior is found, at the weak confinement regime the conduction band minimum and the top of valance band change from s-state to p-state or d-state for confined electron and hole inside IPQD, respectively. The strength of the inverse parabolic potential (potential hump) inside a quantum dot has the upper hand in tuning the ground state momentum for both electron and hole, and consequently their interband transition energy is changed. Knowing that this is not the case for the other types of potentials. The quantum size, the magnetic field and inverse potential hump effects on electron and hole ground and excited states are discussed.
Propagation of surface waves on a semi-bounded quantum magnetized collisional plasma
Niknam, A. R.; Taheri Boroujeni, S.; Khorashadizadeh, S. M.
2013-12-15
The propagation of surface waves on a semi-bounded quantum plasma in the presence of the external magnetic field and collisional effects is investigated by using quantum magnetohydrodynamics model. A general analytical expression for the dispersion relation of surface waves is obtained by considering the boundary conditions. It is shown that, in some special cases, the obtained dispersion relation reduces to the results reported in previous works. It is also indicated that the quantum, external magnetic field and collisional effects can facilitate the propagation of surface waves on a semi-bounded plasma. In addition, it is found that the growth rate of the surface wave instability is enhanced by increasing the collision frequency and plasmonic parameter.
NASA Astrophysics Data System (ADS)
Hayrapetyan, D. B.; Kazaryan, E. M.; Sarkisyan, H. A.
2016-01-01
An electron gas in a strongly oblated ellipsoidal quantum dot with impenetrable walls in the presence of external magnetic field is considered. Influence of the walls of the quantum dot is assumed to be so strong in the direction of the minor axis (the OZ axis) that the Coulomb interaction between electrons in this direction can be neglected and considered as two-dimensional. On the basis of geometric adiabaticity we show that in the case of a few-particle gas a powerful repulsive potential of the quantum dot walls has a parabolic form and localizes the gas in the geometric center of the structure. Due to this fact, conditions occur to implement the generalized Kohn theorem for this system. The parabolic confinement potential depends on the geometry of the ellipsoid, which allows, together with the magnetic field to control resonance frequencies of transitions by changing the geometric dimensions of the QD.
The pressure-induced calcium deposition on crosslinked polyurethanes.
Shunmugakumar, N; Jayabalan, M
1992-06-01
The pressure-induced calcium deposition in crosslinked polyurethane was studied. Two polyurethane systems, IPDI-PTMG/PPG-TMP and SMDI-PTMG/PPG-TMP were subjected to calcification under induced pressure. Calcium deposition in IPDI polymers was linear with the increase of soft segment (PTMG) content whereas in SMDI polymers the reverse trend was observed. Decreased phase mixing and hydrophilicity in the polymer (SMDI based) having increased soft segment content was attributed to the decreased calcification. The enhanced amount of calcium deposition under pressure indicates the possible influence of pressure on calcification. PMID:10078255
NASA Astrophysics Data System (ADS)
Ohanyan, Vadim; Rojas, Onofre; Strečka, Jozef; Bellucci, Stefano
2015-12-01
We examine the general features of the noncommutativity of the magnetization operator and Hamiltonian for small quantum spin clusters. The source of this noncommutativity can be a difference in the Landé g factors for different spins in the cluster, X Y anisotropy in the exchange interaction, and the presence of the Dzyaloshinskii-Moriya term in a direction different from the direction of the magnetic field. As a result, zero-temperature magnetization curves for small spin clusters mimic those for the macroscopic systems with the band(s) of magnetic excitations, i.e., for the given eigenstate of the spin cluster the corresponding magnetic moment can be an explicit function of the external magnetic field yielding the nonconstant (nonplateau) form of the magnetization curve within the given eigenstate. In addition, the X Y anisotropy makes the saturated magnetization (the eigenstate when all spins in cluster are aligned along the magnetic field) inaccessible for finite magnetic field magnitude (asymptotical saturation). We demonstrate all these features on three examples: a spin-1/2 dimer, mixed spin-(1/2,1) dimer, and a spin-1/2 ring trimer. We consider also the simplest Ising-Heisenberg chain, the Ising-X Y Z diamond chain, with four different g factors. In the chain model the magnetization curve has a more complicated and nontrivial structure than that for clusters.
Quantum correlations of magnetic impurities by a multiple electron scattering in carbon nanotubes
NASA Astrophysics Data System (ADS)
Gamboa Angulo, Didier; Cordourier Maruri, Guillermo; de Coss Gómez, Romeo
In this work we analyze the quantum correlations and polarizations states of magnetic impurities spins, when a multiple electron scattering was taken place. A sequence of non-correlated electrons interacts through scattering producing quantum correlation which will have an impact on the electronic transmission. We consider a short range Heisenberg interaction between ballistic electron and static impurities. We analyze the cases when the electron scattering is produce by one and two impurities, obtaining the electronic transmission rates. Concurrence and fidelity calculations are performed to obtain the level of quantum entanglement and polarization correlations. We also discuss the possible application of this model to metallic and semiconductor carbon nanotubes, which could have important implications on spintronics and quantum information devices.
Quantum theory of the dielectric constant of a magnetized plasma and astrophysical applications. I.
NASA Technical Reports Server (NTRS)
Canuto, V.; Ventura, J.
1972-01-01
A quantum mechanical treatment of an electron plasma in a constant and homogeneous magnetic field is considered, with the aim of (1) defining the range of validity of the magnetoionic theory (2) studying the deviations from this theory, in applications involving high densities, and intense magnetic field. While treating the magnetic field exactly, a perturbation approach in the photon field is used to derive general expressions for the dielectric tensor. Numerical estimates on the range of applicability of the magnetoionic theory are given for the case of the 'one-dimensional' electron gas, where only the lowest Landau level is occupied.
NASA Astrophysics Data System (ADS)
Fritsch, K.; Ehlers, G.; Rule, K. C.; Habicht, K.; Ramazanoglu, M.; Dabkowska, H. A.; Gaulin, B. D.
2015-11-01
The application of a magnetic field transverse to the easy axis, Ising direction in the quasi-two-dimensional kagome staircase magnet, Co3V2O8 , induces three quantum phase transitions at low temperatures, ultimately producing a novel high field polarized state, with two distinct sublattices. New time-of-flight neutron scattering techniques, accompanied by large angular access, high magnetic field infrastructure allow the mapping of a sequence of ferromagnetic and incommensurate phases and their accompanying spin excitations. At least one of the transitions to incommensurate phases at μ0Hc 1˜6.25 T and μ0Hc 2˜7 T is discontinuous, while the final quantum critical point at μ0Hc 3˜13 T is continuous.
Fritsch, Katharina; Ehlers, G.; Rule, K. C.; Habicht, Klaus; Ramazanoglu, Mehmet K.; Dabkowska, H. A.; Gaulin, Bruce D.
2015-11-05
We study the application of a magnetic field transverse to the easy axis, Ising direction in the quasi-two-dimensional kagome staircase magnet, Co3V2O8, induces three quantum phase transitions at low temperatures, ultimately producing a novel high field polarized state, with two distinct sublattices. New time-of-flight neutron scattering techniques, accompanied by large angular access, high magnetic field infrastructure allow the mapping of a sequence of ferromagnetic and incommensurate phases and their accompanying spin excitations. Also, at least one of the transitions to incommensurate phases at μ0Hc1~6.25 T and μ0Hc2~7 T is discontinuous, while the final quantum critical point at μ0Hc3~13 T ismore » continuous.« less
NASA Astrophysics Data System (ADS)
Chen, Zhi-De; Liang, J.-Q.; Shen, Shun-Qing
2002-09-01
Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a transverse magnetic field along the hard axis is smeared by the finite distribution, which subsequently affects the quantum steps of the hysteresis curve evaluated in terms of the modified Landau-Zener model of spin flipping induced by the sweeping field. We conclude that the dipolar-dipolar interaction drives decoherence of quantum tunneling in the molecular magnet Fe8, which explains why the quenching points of tunnel splitting between odd and even resonant tunneling predicted theoretically were not observed experimentally.
Quantum melting of magnetic order in an organic dimer Mott-insulating system
NASA Astrophysics Data System (ADS)
Naka, Makoto; Ishihara, Sumio
2016-05-01
Quantum entanglement effects between the electronic spin and charge degrees of freedom are examined in an organic molecular solid, termed a dimer Mott-insulating system, in which molecular dimers are arranged in a crystal as fundamental units. A low energy effective model includes an antisymmetric exchange interaction, as one of the dominant magnetic interactions. This interaction favors a 90 deg spin configuration, and competes with the Heisenberg-type exchange interaction. Stabilities of the magnetic ordered phases are examined by using the spin-wave theory, as well as the Schwinger-boson theory. It is found that the spin-charge interaction promotes an instability of the long-range magnetic ordered state around a parameter region where two spin-spiral phases are merged. Implication for the quantum spin liquid state observed in κ -(BEDT-TTF)2Cu2 (CN) 3 is discussed.
Quantum Magnetism and Topological Ordering via Rydberg Dressing near Förster Resonances.
van Bijnen, R M W; Pohl, T
2015-06-19
We devise a cold-atom approach to realizing a broad range of bilinear quantum magnets. Our scheme is based on off-resonant single-photon excitation of Rydberg P states (Rydberg dressing), whose strong interactions are shown to yield controllable XYZ interactions between effective spins, represented by different atomic ground states. The distinctive features of Förster-resonant Rydberg atom interactions are exploited to enhance the effectiveness of Rydberg dressing and, thereby, yield large spin interactions that greatly exceed the corresponding decoherence rates. We illustrate the concept on a spin-1 chain implemented with cold rubidium atoms, and demonstrate that this permits the dynamical preparation of topological magnetic phases. Generally, the described approach provides a viable route to exploring quantum magnetism with dynamically tunable (an)isotropic interactions as well as variable space and spin dimensions in cold-atom experiments. PMID:26196973
Noiseless manipulation of helical edge state transport by a quantum magnet
NASA Astrophysics Data System (ADS)
Silvestrov, P. G.; Recher, P.; Brouwer, P. W.
2016-05-01
The current through a helical edge state of a quantum spin Hall insulator may be fully transmitted through a magnetically gapped region due to a combination of spin-transfer torque and spin pumping [Meng et al., Phys. Rev. B 90, 205403 (2014), 10.1103/PhysRevB.90.205403]. Using a scattering approach, we here argue that in such a system the current is effectively carried by electrons with energies below the magnet-induced gap and well below the Fermi energy. This has striking consequences, such as the absence of shot noise, an exponential suppression of thermal noise, and an obstruction of thermal transport. For two helical edges covered by the same quantum magnet, the device can act as a robust noiseless current splitter.
Magnetic bead-quantum dot assay for detection of a biomarker for traumatic brain injury.
Kim, Chloe; Searson, Peter C
2015-11-14
Current diagnostic methods for traumatic brain injury (TBI), which accounts for 15% of all emergency room visits, are limited to neuroimaging modalities. The challenges of accurate diagnosis and monitoring of TBI have created the need for a simple and sensitive blood test to detect brain-specific biomarkers. Here we report on an assay for detection of S100B, a putative biomarker for TBI, using antibody-conjugated magnetic beads for capture of the protein, and antibody-conjugated quantum dots for optical detection. From Western Blot, we show efficient antigen capture and concentration by the magnetic beads. Using magnetic bead capture and quantum dot detection in serum samples, we show a wide detection range and detection limit below the clinical cut-off level. PMID:26457768
Magnetic Torque Anomaly in the Quantum Limit of Weyl and Dirac Semimetals
NASA Astrophysics Data System (ADS)
Nair, Nityan L.; Moll, Philip J. W.; Potter, Andrew C.; Ramshaw, Brad; Modic, Kimberly; Riggs, Scott; Zeng, Bin; Ghimire, Nirmal; Bauer, Eric; Kealhofer, Robert; Li, Zhenglu; Louie, Steven; Ronning, Filip; Analytis, James G.
Three dimensional Dirac and Weyl semimetals, characterized by bulk quasiparticles that behave as massless, linearly dispersing Dirac or Weyl fermions, have excited physicists with their unique topological properties and potential for applications. The experimental signatures of Weyl or Dirac fermions, however, are often subtle and indirect, especially in systems where they coexist with trivial electrons. Here, we report a novel method by which these topological systems can be unambiguously experimentally identified. Magnetic torque measurements were performed on the Weyl semimetal NbAs in high magnetic field, showing a large anomaly upon entering the quantum limit. The torque exhibits a striking sign reversal, corresponding to a change in the magnetic anisotropy that is a direct result of the topological properties of the charge carriers. This result can be generalized to other Dirac and Weyl semimetal systems and establishes quantum limit torque measurements as a simple and direct experimental method of distinguishing topologically non-trivial Weyl and Dirac systems from trivial semiconductors.
Nuclear magnetic resonance detection and spectroscopy of single proteins using quantum logic.
Lovchinsky, I; Sushkov, A O; Urbach, E; de Leon, N P; Choi, S; De Greve, K; Evans, R; Gertner, R; Bersin, E; Müller, C; McGuinness, L; Jelezko, F; Walsworth, R L; Park, H; Lukin, M D
2016-02-19
Nuclear magnetic resonance spectroscopy is a powerful tool for the structural analysis of organic compounds and biomolecules but typically requires macroscopic sample quantities. We use a sensor, which consists of two quantum bits corresponding to an electronic spin and an ancillary nuclear spin, to demonstrate room temperature magnetic resonance detection and spectroscopy of multiple nuclear species within individual ubiquitin proteins attached to the diamond surface. Using quantum logic to improve readout fidelity and a surface-treatment technique to extend the spin coherence time of shallow nitrogen-vacancy centers, we demonstrate magnetic field sensitivity sufficient to detect individual proton spins within 1 second of integration. This gain in sensitivity enables high-confidence detection of individual proteins and allows us to observe spectral features that reveal information about their chemical composition. PMID:26847544
Nuclear magnetic resonance detection and spectroscopy of single proteins using quantum logic
NASA Astrophysics Data System (ADS)
Lovchinsky, I.; Sushkov, A. O.; Urbach, E.; de Leon, N. P.; Choi, S.; De Greve, K.; Evans, R.; Gertner, R.; Bersin, E.; Müller, C.; McGuinness, L.; Jelezko, F.; Walsworth, R. L.; Park, H.; Lukin, M. D.
2016-02-01
Nuclear magnetic resonance spectroscopy is a powerful tool for the structural analysis of organic compounds and biomolecules but typically requires macroscopic sample quantities. We use a sensor, which consists of two quantum bits corresponding to an electronic spin and an ancillary nuclear spin, to demonstrate room temperature magnetic resonance detection and spectroscopy of multiple nuclear species within individual ubiquitin proteins attached to the diamond surface. Using quantum logic to improve readout fidelity and a surface-treatment technique to extend the spin coherence time of shallow nitrogen-vacancy centers, we demonstrate magnetic field sensitivity sufficient to detect individual proton spins within 1 second of integration. This gain in sensitivity enables high-confidence detection of individual proteins and allows us to observe spectral features that reveal information about their chemical composition.
Search for pressure-induced superconductivity in CeFeAsO and CeFePO iron pnictides
Zocco, D. A.; Baumbach, R. E.; Hamlin, J. J.; Janoschek, M.; Lum, I. K.; McGuire, Michael A; Safa-Sefat, Athena; Sales, Brian C; Jin, Rongying; Mandrus, David; Jeffries, J. R.; Weir, S. T.; Vohra, Y. K.; Maple, M. B.
2011-01-01
The CeFeAsO and CeFePO iron pnictide compounds were studied via electrical transport measurements under high pressure. In CeFeAsO polycrystals, the magnetic phases involving the Fe and Ce ions coexist for hydrostatically applied pressures up to 15 GPa, and with no signs of pressure-induced superconductivity up to 50 GPa for the less hydrostatic pressure techniques. For the CeFePO single crystals, pressure further stabilizes the Kondo screening of the Ce 4f-electron magnetic moments.
Irreversibility of pressure induced boron speciation change in glass.
Smedskjaer, Morten M; Youngman, Randall E; Striepe, Simon; Potuzak, Marcel; Bauer, Ute; Deubener, Joachim; Behrens, Harald; Mauro, John C; Yue, Yuanzheng
2014-01-01
It is known that the coordination number (CN) of atoms or ions in many materials increases through application of sufficiently high pressure. This also applies to glassy materials. In boron-containing glasses, trigonal BO3 units can be transformed into tetrahedral BO4 under pressure. However, one of the key questions is whether the pressure-quenched CN change in glass is reversible upon annealing below the ambient glass transition temperature (Tg). Here we address this issue by performing (11)B NMR measurements on a soda lime borate glass that has been pressure-quenched at ~0.6 GPa near Tg. The results show a remarkable phenomenon, i.e., upon annealing at 0.9Tg the pressure-induced change in CN remains unchanged, while the pressurised values of macroscopic properties such as density, refractive index, and hardness are relaxing. This suggests that the pressure-induced changes in macroscopic properties of soda lime borate glasses compressed up to ~0.6 GPa are not attributed to changes in the short-range order in the glass, but rather to changes in overall atomic packing density and medium-range structures. PMID:24442182
Irreversibility of Pressure Induced Boron Speciation Change in Glass
Smedskjaer, Morten M.; Youngman, Randall E.; Striepe, Simon; Potuzak, Marcel; Bauer, Ute; Deubener, Joachim; Behrens, Harald; Mauro, John C.; Yue, Yuanzheng
2014-01-01
It is known that the coordination number (CN) of atoms or ions in many materials increases through application of sufficiently high pressure. This also applies to glassy materials. In boron-containing glasses, trigonal BO3 units can be transformed into tetrahedral BO4 under pressure. However, one of the key questions is whether the pressure-quenched CN change in glass is reversible upon annealing below the ambient glass transition temperature (Tg). Here we address this issue by performing 11B NMR measurements on a soda lime borate glass that has been pressure-quenched at ~0.6 GPa near Tg. The results show a remarkable phenomenon, i.e., upon annealing at 0.9Tg the pressure-induced change in CN remains unchanged, while the pressurised values of macroscopic properties such as density, refractive index, and hardness are relaxing. This suggests that the pressure-induced changes in macroscopic properties of soda lime borate glasses compressed up to ~0.6 GPa are not attributed to changes in the short-range order in the glass, but rather to changes in overall atomic packing density and medium-range structures. PMID:24442182
Magnetic bead-quantum dot assay for detection of a biomarker for traumatic brain injury
NASA Astrophysics Data System (ADS)
Kim, Chloe; Searson, Peter C.
2015-10-01
Current diagnostic methods for traumatic brain injury (TBI), which accounts for 15% of all emergency room visits, are limited to neuroimaging modalities. The challenges of accurate diagnosis and monitoring of TBI have created the need for a simple and sensitive blood test to detect brain-specific biomarkers. Here we report on an assay for detection of S100B, a putative biomarker for TBI, using antibody-conjugated magnetic beads for capture of the protein, and antibody-conjugated quantum dots for optical detection. From Western Blot, we show efficient antigen capture and concentration by the magnetic beads. Using magnetic bead capture and quantum dot detection in serum samples, we show a wide detection range and detection limit below the clinical cut-off level.Current diagnostic methods for traumatic brain injury (TBI), which accounts for 15% of all emergency room visits, are limited to neuroimaging modalities. The challenges of accurate diagnosis and monitoring of TBI have created the need for a simple and sensitive blood test to detect brain-specific biomarkers. Here we report on an assay for detection of S100B, a putative biomarker for TBI, using antibody-conjugated magnetic beads for capture of the protein, and antibody-conjugated quantum dots for optical detection. From Western Blot, we show efficient antigen capture and concentration by the magnetic beads. Using magnetic bead capture and quantum dot detection in serum samples, we show a wide detection range and detection limit below the clinical cut-off level. Electronic supplementary information (ESI) available. See DOI: 10.1039/c5nr05608j
NASA Astrophysics Data System (ADS)
Kharkov, Yaroslav; Oleg P Sushkov Team
We consider two spin 1 / 2 fermions in a two-dimensional magnetic system that is close to the O (3) magnetic quantum critical point (QCP) which separates magnetically ordered and disordered phases. Focusing on the disordered phase in the vicinity of the QCP, we demonstrate that the criticality results in a strong long range attraction between the fermions, with potential V (r) ~ - 1 /rα , α ~ 0 . 75 , where r is separation between the fermions. The mechanism of the enhanced attraction is similar to Casimir effect and corresponds to multi-magnon exchange processes between the fermions. While we consider a model system, the problem is originally motivated by recent experimental establishment of magnetic QCP in hole doped cuprates under the superconducting dome at doping of about 10%. We suggest the mechanism of magnetic critical enhancement of pairing in cuprates.
Yang, Jiehui; Ma, Shengcan; Xu, You
2009-03-01
The pronounced anisotropy of the magnetization caused by the Ho(3+) ions in the ferrimagnetic holmium iron garnet has been investigated based on quantum theory. The strong anisotropy of the magnetization of the Ho(3+) ions originates mainly from the effect of the crystal field upon the Ho(3+) ions and the anisotropic Ho(3+)-Fe(3+) superexchange interaction. Following the expression of the Yb(3+)-Fe(3+) exchange interaction used by Alben, the anisotropy of the Ho(3+)-Fe(3+) exchange interaction is defined by three principal values of the exchange tensor G. Because the six Ho(3+) sublattices are magnetically non-equivalent, we calculate the magnetic quantities of the Ho(3+) at the six sublattices and compare the average value of the so-obtained six quantities with the measured values. The calculated results are in good agreement with experiments. An interpretation on the anisotropy of the magnetic properties of HoIG is given. PMID:21817410
Magnetic enhancement of photoluminescence from blue-luminescent graphene quantum dots
NASA Astrophysics Data System (ADS)
Chen, Qi; Shi, Chentian; Zhang, Chunfeng; Pu, Songyang; Wang, Rui; Wu, Xuewei; Wang, Xiaoyong; Xue, Fei; Pan, Dengyu; Xiao, Min
2016-02-01
Graphene quantum-dots (GQDs) have been predicted and demonstrated with fascinating optical and magnetic properties. However, the magnetic effect on the optical properties remains experimentally unexplored. Here, we conduct a magneto-photoluminescence study on the blue-luminescence GQDs at cryogenic temperatures with magnetic field up to 10 T. When the magnetic field is applied, a remarkable enhancement of photoluminescence emission has been observed together with an insignificant change in circular polarization. The results have been well explained by the scenario of magnetic-field-controlled singlet-triplet mixing in GQDs owing to the Zeeman splitting of triplet states, which is further verified by temperature-dependent experiments. This work uncovers the pivotal role of intersystem crossing in GQDs, which is instrumental for their potential applications such as light-emitting diodes, photodynamic therapy, and spintronic devices.
NASA Astrophysics Data System (ADS)
Kalmykov, Yuri P.; Titov, Serguey V.; Coffey, William T.
2015-11-01
The nonlinear ac stationary response of uniaxial paramagnets and superparamagnets—nanoscale solids or clusters with spin number S ˜100-104 —in superimposed uniform ac and dc bias magnetic fields of arbitrary strength, each applied along the easy axis of magnetization, is determined by solving the evolution equation for the reduced density matrix represented as a finite set of three-term differential-recurrence relations for its diagonal matrix elements. The various harmonic components arising from the nonlinear response of the magnetization, dynamic magnetic hysteresis loops, etc., are then evaluated via matrix continued fractions indicating a pronounced dependence of the response on S arising from the quantum spin dynamics, which differ markedly from the magnetization dynamics of classical nanomagnets. In the linear response approximation, the results concur with existing solutions.
NASA Astrophysics Data System (ADS)
Pelliccione, Matthew; Jenkins, Alec; Ovartchaiyapong, Preeti; Reetz, Christopher; Emmanuelidu, Eve; Ni, Ni; Bleszynski Jayich, Ania
The nitrogen vacancy (NV) defect in diamond has emerged as a promising candidate for high resolution magnetic imaging based on its atomic size and quantum-limited sensing capabilities afforded by long spin coherence times. Although the NV center has been successfully implemented as a nanoscale scanning magnetic probe at room temperature, it has remained an outstanding challenge to extend this capability to cryogenic temperatures, where many solid-state systems exhibit non-trivial magnetic order. In this talk, we present NV magnetic imaging at T = 6 K, first benchmarking the technique with a magnetic hard disk sample, then utilizing the technique to image vortices in the iron pnictide superconductor BaFe2(As0.7P0.3)2 with Tc = 30 K. In addition, we discuss other candidate solid-state systems that can benefit from the high spatial resolution and field sensitivity of the scanning NV magnetometer.
Magnetic compasses in biological systems: Does quantum physics play a role?
NASA Astrophysics Data System (ADS)
Ritz, Thorsten
2011-03-01
One hypothesis of the process underlying the magnetic compass of animals surmises that the magnetic field is perceived by its effect on the coherent spin evolution within a non-equilibrium photochemical radical pair reaction. If this hypothesis were proven, it would be a dramatic demonstration of a quantum process with clear biological significance. We will review the physics of the radical pair mechanism and the current state of evidence supporting it. Experimentally, we will focus on the use radio-frequency magnetic fields to affect a radical-pair based mechanism in birds and discuss the approach and its limitations. Theoretically, we will focus on the question of how one should design a radical pair to be optimally sensitive to the direction of a weak magnetic field. Regardless of whether or not a radical pair mechanism is indeed used by birds or other animals, optimal design features could be used to manufacture biologically inspired, but man-made magnetic compass systems.
The quantum equations of state of plasma under the influence of a weak magnetic field
Hussein, N. A.; Eisa, D. A.; Eldin, M. G.
2012-05-15
The aim of this paper is to calculate the magnetic quantum equations of state of plasma, the calculation is based on the magnetic binary Slater sum in the case of low density. We consider only the thermal equilibrium plasma in the case of n{lambda}{sub ab}{sup 3} Much-Less-Than 1, where {lambda}{sub ab}{sup 2}=( Planck-Constant-Over-Two-Pi {sup 2}/m{sub ab}KT) is the thermal De Broglie wave length between two particles. The formulas contain the contributions of the magnetic field effects. Using these results we compute the magnetization and the magnetic susceptibility. Our equation of state is compared with others.
Magnetic moments of light nuclei from lattice quantum chromodynamics
Beane, S. R.; Chang, E.; Cohen, S.; Detmold, W.; Lin, H. W.; Orginos, K.; Parreño, A.; Savage, M. J.; Tiburzi, B. C.
2014-12-16
We present the results of lattice QCD calculations of the magnetic moments of the lightest nuclei, the deuteron, the triton and 3He, along with those of the neutron and proton. These calculations, performed at quark masses corresponding to mπ ~ 800 MeV, reveal that the structure of these nuclei at unphysically heavy quark masses closely resembles that at the physical quark masses. We find that the magnetic moment of 3He differs only slightly from that of a free neutron, as is the case in nature, indicating that the shell-model configuration of two spin-paired protons and a valence neutron captures itsmore » dominant structure. Similarly a shell-model-like moment is found for the triton, μ3H ~ μp. The deuteron magnetic moment is found to be equal to the nucleon isoscalar moment within the uncertainties of the calculations.« less
Decoherence in Quantum Magnets: Theory and Experiment on T2
NASA Astrophysics Data System (ADS)
Tupitsyn, Igor; Stamp, Philip; Takahashi, Susumu; Sherwin, Mark; van Tol, Johan; Beedle, Christopher; Hendrickson, David
2010-03-01
The individual properties of molecular magnets are controlled by chemistry rather than nanoengineering, and are highly tunable. This makes them ideal candidates for solid-state qubits. However decoherence in many solid-state systems is anomalously high, and their advantages cannot be exploited until decoherence is understood and suppressed. In molecular magnets decoherence is caused by coupling to the nuclear spin bath, to phonons, and to each other via dipole-dipole and exchange interactions. Here we study decoherence in 2 different crystals of Fe8 nanomolecules, in several field orientations, both theoretically and experimentally. The experimental results for the decoherence time T2 agree with the existing theory (Morello et al., Phys Rev Lett 97, 207206 (2006)). To our knowledge this is the first time that experimental decoherence rates agree with theory in magnetic systems.
Properties of strong-coupling magneto-bipolaron qubit in quantum dot under magnetic field
NASA Astrophysics Data System (ADS)
Xu-Fang, Bai; Ying, Zhang; Wuyunqimuge; Eerdunchaolu
2016-07-01
Based on the variational method of Pekar type, we study the energies and the wave-functions of the ground and the first-excited states of magneto-bipolaron, which is strongly coupled to the LO phonon in a parabolic potential quantum dot under an applied magnetic field, thus built up a quantum dot magneto-bipolaron qubit. The results show that the oscillation period of the probability density of the two electrons in the qubit decreases with increasing electron–phonon coupling strength α, resonant frequency of the magnetic field ω c, confinement strength of the quantum dot ω 0, and dielectric constant ratio of the medium η the probability density of the two electrons in the qubit oscillates periodically with increasing time t, angular coordinate φ 2, and dielectric constant ratio of the medium η the probability of electron appearing near the center of the quantum dot is larger, and the probability of electron appearing away from the center of the quantum dot is much smaller. Project supported by the Natural Science Foundation of Hebei Province, China (Grant No. E2013407119) and the Items of Institution of Higher Education Scientific Research of Hebei Province and Inner Mongolia, China (Grant Nos. ZD20131008, Z2015149, Z2015219, and NJZY14189).
Pressure induced spin transition revealed by iron M{sub 2,3}-edge spectroscopy
Nyrow, Alexander; Büning, Thomas; Mende, Kolja; Tolan, Metin; Sternemann, Christian; Hiraoka, Nozomu; Desgreniers, Serge; Wilke, Max
2014-06-30
We present a method to characterize pressure induced magnetic high to low spin transition in iron sulphide using x-ray Raman scattering spectroscopy at the iron M{sub 2,3}-edge. The advantage of this method is that the observed spectral changes between pressures of 1.7 GPa and 10.1 GPa can be used with the help of atomic multiplet calculations to determine the crystal field splitting parameters associated with the spin transition. We discuss the potential of this M{sub 2,3}-edge spectroscopy to investigate the irons electronic spin state in-situ at the conditions of the inner Earth, i.e., at high temperature and high pressure, providing exciting opportunities for geophysical and materials science applications.
Pressure Induced Local Structure Distortions in Cu(pyz)F2(H2O)2
Musfeldt, J.L.; Carr, G.; Liu, Z.; Li, S.; Kang, C.L., Jena, P.; Manson, J.L.; Schlueter, J.A. Whangbo, M.H.
2011-06-06
We employed infrared spectroscopy along with complementary lattice dynamics and spin density calculations to investigate pressure-driven local structure distortions in the copper coordination polymer Cu(pyz)F{sub 2}(H{sub 2}O){sub 2}. Here, pyz is pyrazine. Our study reveals rich and fully reversible local lattice distortions that buckle the pyrazine ring, disrupt the bc-plane O-H {hor_ellipsis} F hydrogen-bonding network, and reinforce magnetic property switching. The resiliency of the soft organic ring is a major factor in the stability of this material. Interestingly, the collective character of the lattice vibrations masks direct information on the Cu-N and Cu-O linkages through the series of pressure-induced Jahn-Teller axis switching transitions, although Cu-F bond softening is clearly identified above 3 GPa. These findings illustrate the importance of combined bulk and local probe techniques for microscopic structure determination in complex materials.
Pressure-Induced Local Structure Distortions in Cu(pyz)F(2)(H(2)O)(2)
J Musfeldt; Z Liu; S Li; J Kang; C Lee; P Jena; J Manson; J Schlueter; G Carr; M Whangbo
2011-12-31
We employed infrared spectroscopy along with complementary lattice dynamics and spin density calculations to investigate pressure-driven local structure distortions in the copper coordination polymer Cu(pyz)F{sub 2}(H{sub 2}O){sub 2}. Here, pyz is pyrazine. Our study reveals rich and fully reversible local lattice distortions that buckle the pyrazine ring, disrupt the bc-plane O-H {hor_ellipsis} F hydrogen-bonding network, and reinforce magnetic property switching. The resiliency of the soft organic ring is a major factor in the stability of this material. Interestingly, the collective character of the lattice vibrations masks direct information on the Cu-N and Cu-O linkages through the series of pressure-induced Jahn-Teller axis switching transitions, although Cu-F bond softening is clearly identified above 3 GPa. These findings illustrate the importance of combined bulk and local probe techniques for microscopic structure determination in complex materials.
Observation of the transition state for pressure-induced BO₃→ BO₄ conversion in glass.
Edwards, Trenton; Endo, Takatsugu; Walton, Jeffrey H; Sen, Sabyasachi
2014-08-29
A fundamental mechanistic understanding of the pressure- and/or temperature-induced facile transformation of the coordination environment of boron is important for changing the physical properties of glass. We have used in situ high-pressure (up to 2 gigapascals) boron-11 solid-state nuclear magnetic resonance spectroscopy in combination with ab initio calculations to investigate the nature of the transition state for the pressure-induced BO3→ BO4 conversion in a borosilicate glass at ambient temperature. The results indicate an anisotropic elastic deformation of the BO3 planar triangle, under isotropic stress, into a trigonal pyramid that likely serves as a precursor for the subsequent formation of a BO4 tetrahedron. PMID:25170146
Multiple quantum filtering and spin exchange in solid state nuclear magnetic resonance
NASA Astrophysics Data System (ADS)
Ba, Yong; Ripmeester, John A.
1998-05-01
Multiple quantum NMR of coupled spin-1/2 nuclei in a solid has been exploited as a filter to separate different magnetization components in a spatially heterogeneous system. After filtering, the spins labeled according to coherence orders were used to follow the track of spin exchange between different domains. In order to avoid time-consuming two-dimensional experiments, this exchange was detected in a one-dimensional experiment via selective detection of multiple quantum coherences. The technique was demonstrated for samples of solid adamantane in contact with its saturated solution in benzene-d6 and for a high-density polyoxymethylene.
Measurement of the Magnetic Flux Noise Spectrum in Superconducting Xmon Transmon Quantum Bits
NASA Astrophysics Data System (ADS)
Chiaro, Ben; Sank, D.; Kelly, J.; Chen, Z.; Campbell, B.; Dunsworth, A.; O'Malley, P.; Neill, C.; Quintana, C.; Vainsencher, A.; Wenner, J.; Barends, R.; Chen, Y.; Fowler, A.; Jeffrey, E.; Migrant, A.; Mutus, J.; Roushan, P.; White, T.; Martinis, J. M.
Dephasing induced by magnetic flux noise limits the performance of modern superconducting quantum processors. We measure the flux noise power spectrum in planar, frequency-tunable, Xmon transmon quantum bits (qubits), with several SQUID loop geometries. We extend the Ramsey Tomography Oscilloscope (RTO) technique by rapid sampling up to 1 MHz, without state reset, to measure the flux noise power spectrum between 10-2 and 105 Hz. The RTO measurements are combined with idle gate randomized benchmarking and Ramsey decay to give a more complete picture of dephasing in SQUID-based devices.
Electron motion induced by magnetic pulse in a bilayer quantum wire
NASA Astrophysics Data System (ADS)
Chwiej, T.
2016-06-01
We consider theoretical stimulation of electron motion in a quantum wire by means of ultrashort magnetic pulses of time duration between several and a few tens of picoseconds. In our considerations, an electron is confined in a nanowire which consists of two vertically stacked tunnel-coupled layers. If a magnetic pulse pierces this nanowire and its direction is parallel to the plane established by the layers, and additionally, it is perpendicular to the wire's axis, then the eigenstates of a single electron energy operator for vertical direction are hybridized by the off-diagonal terms of the full Hamiltonian. These terms depend linearly on the momentum operator, which means that such magnetically forced hybridization may induce electron motion in a nanowire. The classical counterpart of this quantum-mechanical picture is a situation in which the rotational electric field generated by a time-varying magnetic field pushes the charge densities localized in the upper and lower layers in opposite directions. We have found, however, that for an asymmetric vertical confinement in a bilayer nanowire, the major part of the single electron density starts to move in the direction of the local electric field in its layer forcing the minority part to move in this direction as well. It results in coherent motion of both densities in a particular direction. We analyze the dynamics of such motion in dependence on the time characteristics of a magnetic pulse and discuss potential applications of this effect in the construction of a magnetic valve.
NASA Astrophysics Data System (ADS)
Mogi, M.; Yoshimi, R.; Tsukazaki, A.; Yasuda, K.; Kozuka, Y.; Takahashi, K. S.; Kawasaki, M.; Tokura, Y.
2015-11-01
Quantum anomalous Hall effect (QAHE), which generates dissipation-less edge current without external magnetic field, is observed in magnetic-ion doped topological insulators (TIs) such as Cr- and V-doped (Bi,Sb)2Te3. The QAHE emerges when the Fermi level is inside the magnetically induced gap around the original Dirac point of the TI surface state. Although the size of gap is reported to be about 50 meV, the observable temperature of QAHE has been limited below 300 mK. We attempt magnetic-Cr modulation doping into topological insulator (Bi,Sb)2Te3 films to increase the observable temperature of QAHE. By introducing the rich-Cr-doped thin (1 nm) layers at the vicinity of both the surfaces based on non-Cr-doped (Bi,Sb)2Te3 films, we have succeeded in observing the QAHE up to 2 K. The improvement in the observable temperature achieved by this modulation-doping appears to be originating from the suppression of the disorder in the surface state interacting with the rich magnetic moments. Such a superlattice designing of the stabilized QAHE may pave a way to dissipation-less electronics based on the higher-temperature and zero magnetic-field quantum conduction.
Mogi, M. Yoshimi, R.; Yasuda, K.; Kozuka, Y.; Tsukazaki, A.; Takahashi, K. S.; Kawasaki, M.; Tokura, Y.
2015-11-02
Quantum anomalous Hall effect (QAHE), which generates dissipation-less edge current without external magnetic field, is observed in magnetic-ion doped topological insulators (TIs) such as Cr- and V-doped (Bi,Sb){sub 2}Te{sub 3}. The QAHE emerges when the Fermi level is inside the magnetically induced gap around the original Dirac point of the TI surface state. Although the size of gap is reported to be about 50 meV, the observable temperature of QAHE has been limited below 300 mK. We attempt magnetic-Cr modulation doping into topological insulator (Bi,Sb){sub 2}Te{sub 3} films to increase the observable temperature of QAHE. By introducing the rich-Cr-doped thin (1 nm) layers at the vicinity of both the surfaces based on non-Cr-doped (Bi,Sb){sub 2}Te{sub 3} films, we have succeeded in observing the QAHE up to 2 K. The improvement in the observable temperature achieved by this modulation-doping appears to be originating from the suppression of the disorder in the surface state interacting with the rich magnetic moments. Such a superlattice designing of the stabilized QAHE may pave a way to dissipation-less electronics based on the higher-temperature and zero magnetic-field quantum conduction.
Singh, Saurabh Kumar; Rajaraman, Gopalan
2016-01-01
Single-molecule magnets represent a promising route to achieve potential applications such as high-density information storage and spintronics devices. Among others, 4d/5d elements such as Re(IV) ion are found to exhibit very large magnetic anisotropy, and inclusion of this ion-aggregated clusters yields several attractive molecular magnets. Here, using ab intio calculations, we unravel the source of giant magnetic anisotropy associated with the Re(IV) ions by studying a series of mononuclear Re(IV) six coordinate complexes. The low-lying doublet states are found to be responsible for large magnetic anisotropy and the sign of the axial zero-field splitting parameter (D) can be categorically predicted based on the position of the ligand coordination. Large transverse anisotropy along with large hyperfine interactions opens up multiple relaxation channels leading to a fast quantum tunnelling of the magnetization (QTM) process. Enhancing the Re-ligand covalency is found to significantly quench the QTM process. PMID:26883278
Singh, Saurabh Kumar; Rajaraman, Gopalan
2016-01-01
Single-molecule magnets represent a promising route to achieve potential applications such as high-density information storage and spintronics devices. Among others, 4d/5d elements such as Re(IV) ion are found to exhibit very large magnetic anisotropy, and inclusion of this ion-aggregated clusters yields several attractive molecular magnets. Here, using ab intio calculations, we unravel the source of giant magnetic anisotropy associated with the Re(IV) ions by studying a series of mononuclear Re(IV) six coordinate complexes. The low-lying doublet states are found to be responsible for large magnetic anisotropy and the sign of the axial zero-field splitting parameter (D) can be categorically predicted based on the position of the ligand coordination. Large transverse anisotropy along with large hyperfine interactions opens up multiple relaxation channels leading to a fast quantum tunnelling of the magnetization (QTM) process. Enhancing the Re-ligand covalency is found to significantly quench the QTM process. PMID:26883278
NASA Astrophysics Data System (ADS)
Singh, Saurabh Kumar; Rajaraman, Gopalan
2016-02-01
Single-molecule magnets represent a promising route to achieve potential applications such as high-density information storage and spintronics devices. Among others, 4d/5d elements such as Re(IV) ion are found to exhibit very large magnetic anisotropy, and inclusion of this ion-aggregated clusters yields several attractive molecular magnets. Here, using ab intio calculations, we unravel the source of giant magnetic anisotropy associated with the Re(IV) ions by studying a series of mononuclear Re(IV) six coordinate complexes. The low-lying doublet states are found to be responsible for large magnetic anisotropy and the sign of the axial zero-field splitting parameter (D) can be categorically predicted based on the position of the ligand coordination. Large transverse anisotropy along with large hyperfine interactions opens up multiple relaxation channels leading to a fast quantum tunnelling of the magnetization (QTM) process. Enhancing the Re-ligand covalency is found to significantly quench the QTM process.
An architecture for quantum computation with magnetically trapped Holmium atoms
NASA Astrophysics Data System (ADS)
Saffman, Mark; Hostetter, James; Booth, Donald; Collett, Jeffrey
2016-05-01
Outstanding challenges for scalable neutral atom quantum computation include correction of atom loss due to collisions with untrapped background gas, reduction of crosstalk during state preparation and measurement due to scattering of near resonant light, and the need to improve quantum gate fidelity. We present a scalable architecture based on loading single Holmium atoms into an array of Ioffe-Pritchard traps. The traps are formed by grids of superconducting wires giving a trap array with 40 μm period, suitable for entanglement via long range Rydberg gates. The states | F = 5 , M = 5 > and | F = 7 , M = 7 > provide a magic trapping condition at a low field of 3.5 G for long coherence time qubit encoding. The F = 11 level will be used for state preparation and measurement. The availability of different states for encoding, gate operations, and measurement, spectroscopically isolates the different operations and will prevent crosstalk to neighboring qubits. Operation in a cryogenic environment with ultra low pressure will increase atom lifetime and Rydberg gate fidelity by reduction of blackbody induced Rydberg decay. We will present a complete description of the architecture including estimates of achievable performance metrics. Work supported by NSF award PHY-1404357.
Terahertz excitations in the 1D Ising chain quantum magnet CoNb2O6
NASA Astrophysics Data System (ADS)
Morris, Christopher M.; Valdés Aguilar, R.; Koopayeh, S.; Broholm, C.; Armitage, N. P.
2012-02-01
The one-dimensional magnet CoNb2O6 was recently demonstrated to be an excellent realization of a one-dimensional quantum Ising spin chain. It has been shown to undergo a quantum phase transition in a magnetic field oriented transverse to its ferromagnetically aligned spin chains. Low energy spin-flip excitations in the chains were recently observed via inelastic neutron scattering.ootnotetextR. Coldea, et al, Science 327, 177 (2010) The energy spectrum of these excitations was shown to have a interesting energy scaling governed by symmetries of the E8 exceptional Lie group. Here, time-domain terahertz spectroscopy (TDTS) is used to investigate optically active low energy excitations in CoNb2O6. We take advantage of the polarization sensitivity of this technique to characterize both electric and magnetic dipole active excitations in this compound. A connection is made from the q=0 response observed here to the excitations observed by neutron scattering. In addition, we will show preliminary data on the terahertz spectra of this material as it undergoes the magnetic field-tuned quantum phase transition.
Fe Doped CdTeS Magnetic Quantum Dots for Bioimaging†
Saha, Ajoy K.; Sharma, Parvesh; Sohn, Han-Byul; Ghosh, Siddhartha; Das, Ritesh. K.; Hebard, Arthur F.; Zeng, Huadong; Baligand, Celine; Walter, Glenn A.
2013-01-01
A facile synthesis of 3-6 nm, water dispersible, near-infrared (NIR) emitting, quantum dots (QDs) magnetically doped with Fe is presented. Doping of alloyed CdTeS nanocrystals with Fe was achieved in situ using a simple hydrothermal method. The magnetic quantum dots (MQDs) were capped with NAcetyl-Cysteine (NAC) ligands, containing thiol and carboxylic acid functional groups to provide stable aqueous dispersion. The optical and magnetic properties of the Fe doped MQDs were characterized using several techniques. The synthesized MQDs are tuned to emit in the Vis-NIR (530-738 nm) wavelength regime and have high quantum yields (67.5-10%). NIR emitting (738 nm) MQDs having 5.6 atomic% Fe content exhibited saturation magnetization of 85 emu/gm[Fe] at room temperature. Proton transverse relaxivity of the Fe doped MQDs (738 nm) at 4.7 T was determined to be 3.6 mM−1s−1. The functional evaluation of NIR MQDs has been demonstrated using phantom and in vitro studies. These water dispersible, NIR emitting and MR contrast producing Fe doped CdTeS MQDs, in unagglomerated form, have the potential to act as multimodal contrast agents for tracking live cells. PMID:24634776
Magnetically induced pumping and memory storage in quantum rings
NASA Astrophysics Data System (ADS)
Cini, Michele; Perfetto, Enrico
2011-12-01
Nanoscopic rings pierced by external magnetic fields and asymmetrically connected to wires behave in sharp contrast with classical expectations. By studying the real-time evolution of tight-binding models in different geometries, we show that the creation of a magnetic dipole by a bias-induced current is a process that can be reversed: connected rings excited by an internal ac flux produce ballistic currents in the external wires. In particular we point out that by employing suitable flux protocols, single-parameter nonadiabatic pumping can be achieved, and an arbitrary amount of charge can be transferred from one side to the other. We also propose a setup that could serve a memory device, in which both the operations of writing and erasing can be efficiently performed.
Magnetic moments of light nuclei from lattice quantum chromodynamics
Beane, S. R.; Chang, E.; Cohen, S.; Detmold, W.; Lin, H. W.; Orginos, K.; Parreño, A.; Savage, M. J.; Tiburzi, B. C.
2014-12-16
We present the results of lattice QCD calculations of the magnetic moments of the lightest nuclei, the deuteron, the triton and ^{3}He, along with those of the neutron and proton. These calculations, performed at quark masses corresponding to m_{π} ~ 800 MeV, reveal that the structure of these nuclei at unphysically heavy quark masses closely resembles that at the physical quark masses. We find that the magnetic moment of ^{3}He differs only slightly from that of a free neutron, as is the case in nature, indicating that the shell-model configuration of two spin-paired protons and a valence neutron captures its dominant structure. Similarly a shell-model-like moment is found for the triton, μ_{3H} ~ μ_{p}. The deuteron magnetic moment is found to be equal to the nucleon isoscalar moment within the uncertainties of the calculations.
Radiation pressure induced difference-sideband generation beyond linearized description
NASA Astrophysics Data System (ADS)
Xiong, Hao; Fan, Yu-Wan; Yang, Xiaoxue; Wu, Ying
2016-08-01
We investigate radiation-pressure induced generation of the frequency components at the difference-sideband in an optomechanical system, which beyond the conventional linearized description of optomechanical interactions between cavity fields and the mechanical oscillation. We analytically calculate amplitudes of these signals, and identify a simple square-root law for both the upper and lower difference-sideband generation which can describe the dependence of the intensities of these signals on the pump power. Further calculation shows that difference-sideband generation can be greatly enhanced via achieving the matching conditions. The effect of difference-sideband generation, which may have potential application for manipulation of light, is especially suited for on-chip optomechanical devices, where nonlinear optomechanical interaction in the weak coupling regime is within current experimental reach.
Pressure-induced phase transformation of In2Se3
NASA Astrophysics Data System (ADS)
Rasmussen, Anya; Teklemichael, Samuel; Mafi, Elham; Gu, Yi; McCluskey, Matthew
2013-06-01
Phase-change memory, with fast read-write speeds and small dimensions, will soon replace flash memory in our cell phones and tablets. This type of memory relies on phase change materials like indium selenide, In2Se3, a III-VI semiconductor that exists in multiple crystalline phases. To achieve controlled switching between phases, it is important to understand both the thermal and elastic properties of In2Se3. Using synchrotron x-ray diffraction and a diamond-anvil cell, a pressure-induced phase transition in powder In2Se3 from the α phase to β phase was discovered at 0.7 GPa. This pressure is an order of magnitude lower than phase-transition pressures in most semiconductors. Raman spectroscopy experiments confirm this result. The bulk moduli are reported for both α and β phases, and the c / a ratio for the β phase is shown to have a nonlinear dependence on pressure.
Atomistic pathways of the pressure-induced densification of quartz
NASA Astrophysics Data System (ADS)
Liang, Yunfeng; Miranda, Caetano R.; Scandolo, Sandro
2015-10-01
When quartz is compressed at room temperature it retains its crystal structure at pressures well above its stability domain (0-2 GPa), and collapses into denser structures only when pressure reaches 20 GPa. Depending on the experimental conditions, pressure-induced densification can be accompanied by amorphization; by the formation of crystalline, metastable polymorphs; and can be preceded by the appearance of an intermediate phase, quartz II, with unknown structure. Based on molecular dynamic simulations, we show that this rich phenomenology can be rationalized through a unified theoretical framework of the atomistic pathways leading to densification. The model emphasizes the role played by the oxygen sublattice, which transforms from a bcc-like order in quartz into close-packed arrangements in the denser structures, through a ferroelastic instability of martensitic nature.
Pressure-induced phase transition in CrO2.
Alptekin, Sebahaddin
2015-12-01
The ab initio constant pressure molecular dynamics technique and density functional theory with generalized gradient approximation (GGA) was used to study the pressure-induced phase transition of CrO2. The phase transition of the rutile (P42/mnm) to the orthorhombic CaCl2 (Pnnm) structure at 30 GPa was determined successfully in a constant pressure simulation. This phase transition was analyzed from total energy calculations and, from the enthalpy calculation, occurred at around 17 GPa. Structural properties such as bulk modules, lattice parameters and phase transition were compared with experimental results. The phase transition at 12 ± 3 GPa was in good agreement with experimental results, as was the phase transition from the orthorhombic CaCl2 (Pnnm) to the monoclinic (P21/c) structure also found at 35 GPa. PMID:26541468
Spin quantum Hall effects in featureless nonfractionalized spin-1 magnets
NASA Astrophysics Data System (ADS)
Lu, Yuan-Ming; Lee, Dung-Hai
2014-05-01
The Affleck-Kennedy-Lieb-Tasaki state (or Haldane phase) in a spin-1 chain represents a large class of gapped topological paramagnets that host symmetry-protected gapless excitations on the boundary. In this work, we show how to realize this type of featureless spin-1 state on a generic two-dimensional lattice. These states have a gapped spectrum in the bulk, but they support gapless edge states protected by spin rotational symmetry along a certain direction, and they exhibit the spin quantum Hall effect. Using a fermion representation of integer spins, we show a concrete example of such spin-1 topological paramagnets on a kagome lattice, and we suggest a microscopic spin-1 Hamiltonian that may realize it.
NASA Astrophysics Data System (ADS)
Binz, Ernst; Schempp, Walter
2001-06-01
Quantum holography is a well established theory of mathematical physics based on harmonic analysis on the Heisenberg Lie group G. The geometric quantization is performed by projectivization of the complexified coadjoint orbit picture of the unitary dual Ĝ of G in order to achieve a geometric adjustment of the quantum scenario to special relativity theory. It admits applications to various imaging modalities such as synthetic aperture radar (SAR) in the microwave range, and, most importantly for the field of non-invasive medical diagnosis, to the clinical imaging modality of magnetic resonance tomography (MRI) in the radio frequency range. Quantum holography explains the quantum teleportation phenomemon through Einstein-Podolsky-Rosen (EPR) channels which is a consequence of the non-locality of phase coherent quantum field theory, the concept of absolute simultaneity of special relativity theory which provides the Einstein equivalence of energy and Fitzgerald-Lorentz dilated mass, and the perfect quantum holographic replication process of molecular genetic information processing. It specifically reveals what was before unobservable in quantum optics, namely the interference phenomena of matter wavelets of Bose-Einstein condensates, and what was before unobservable in special relativity, namely the light in flight (LIF) recording processing by ultrafast laser pulse trains. Finally, it provides a Lie group theoretical approach to the Kruskal coordinatized Schwarzschild manifold of relativistic cosmology with large scale applications to general relativity theory such as gravitational instanton symmetries and the theory of black holes. The direct spinorial detection of gravitational wavelets emitted by the binary radio pulsar PSR 1913+16 and known only by anticipatory system computation so far will also be based on the principles of quantum holography applied to very large array (VLA) radio interferometers. .
Dynamical mass generation in strongly coupled quantum electrodynamics with weak magnetic fields
Ayala, Alejandro; Raya, Alfredo; Rojas, Eduardo; Bashir, Adnan
2006-05-15
We study the dynamical generation of masses for fundamental fermions in quenched quantum electrodynamics in the presence of weak magnetic fields using Schwinger-Dyson equations. Contrary to the case where the magnetic field is strong, in the weak field limit the coupling should exceed certain critical value in order for the generation of masses to take place, just as in the case where no magnetic field is present. The weak field limit is defined as eB<
Magnetic and Ising quantum phase transitions in a model for isoelectronically tuned iron pnictides
NASA Astrophysics Data System (ADS)
Wu, Jianda; Si, Qimiao; Abrahams, Elihu
2016-03-01
Considerations of the observed bad-metal behavior in Fe-based superconductors led to an early proposal for quantum criticality induced by isoelectronic P for As doping in iron arsenides, which has since been experimentally confirmed. We study here an effective model for the isoelectronically tuned pnictides using a large-N approach. The model contains antiferromagnetic and Ising-nematic order parameters appropriate for J1-J2 exchange-coupled local moments on an Fe square lattice, and a damping caused by coupling to itinerant electrons. The zero-temperature magnetic and Ising transitions are concurrent and essentially continuous. The order-parameter jumps are very small, and are further reduced by the interplane coupling; consequently, quantum criticality occurs over a wide dynamical range. Our results reconcile recent seemingly contradictory experimental observations concerning the quantum phase transition in the P-doped iron arsenides.
Quantum and Classical Description of H Atom Under Magnetic Field and Quadrupole Trap Potential
Mahecha, J.; Salas, J. P.
2006-12-01
A discussion regarding the energy levels spectrum of quantum systems whose classical analogous has states of chaotic motion is presented. The chaotic dynamics of the classical underlying system has its manifestation in the wave functions (in the form of 'scars') and in the energy levels (in the form of 'statistical repulsion' of the energy levels). The above mentioned signatures are named 'quantum chaos'. A typical study of quantum chaos requires finding accurate energy eigenvalues of highly excited states, to calculate the nearest neighbors spacing between levels, to perform the 'unfolding' of the spectrum in order to separate the fluctuations, and finally to find the probability distribution of the unfolded spectrum. This is exemplified by the hydrogen atom under uniform magnetic field and a quadrupole electric field.
Quantum capacitance oscillations in graphene under crossed magnetic and electric fields
NASA Astrophysics Data System (ADS)
Alisultanov, Z. Z.; Reis, M. S.
2016-01-01
Quantum oscillations of metallic systems at low temperatures are one of the key rules to experimentally access their electronic properties, such as energy spectrum, scattering mechanisms, geometry of Fermi surface and many other features. The importance of these knowledge is enormous, since from these a thorough understanding of the anomalous Hall effect, thermopower and Nernst coefficients, just to name a few, is possible; and from those knowledge, plenty of applications arise as emerging technologies. In this direction, the present contribution focuses on a complete description of quantum capacitance oscillations of monolayer and bilayer graphene under crossed electric and magnetic fields, considering to this purpose the Lifshitz-Onsager quantization condition. We found a closed theoretical expression for the quantum capacitance and highlight their amplitude, period and phase —important parameters to access the electronic properties of graphene. These results open doors for further experimental studies.
Macroscopic quantum tunneling in small Josephson junctions in a magnetic field.
Ovchinnikov, Yu. N.; Barone, A.; Varlamov, A. A.; Materials Science Division; Max-Planck Inst. for Physics of Complex Systems; Landau Inst. Theoretical Physics; Univ. di Napoli Federico II; Coherentia-INFM, CNR
2007-01-01
We study the phenomenon of macroscopic quantum tunneling (MQT) in small Josephson junctions (JJ) with an externally applied magnetic field. The latter results in the appearance of the Fraunhofer type modulation of the current density along the barrier. The problem of MQT for a pointlike JJ is reduced to the motion of the quantum particle in the washboard potential. In the case of a finite size JJ under consideration, this problem corresponds to a MQT in a potential which itself, besides the phase, depends on space variables. The general expression for the crossover temperature To between thermally activated and macroscopic quantum tunneling regimes and the escaping time {tau}{sub esc} have been calculated.
Quantum critical dynamics of a magnetic impurity in a semiconducting host
NASA Astrophysics Data System (ADS)
Dasari, Nagamalleswararao; Acharya, Swagata; Taraphder, A.; Moreno, Juana; Jarrell, Mark; Vidhyadhiraja, N. S.; N. S. Vidhyadhiraja Collaboration, Prof.; Mark Jarrell Collaboration, Prof.; A. Taraphder Collaboration, Prof.
We have investigated the finite temperature dynamics of the singlet to doublet continuous quantum phase transition in the gapped Anderson impurity model using hybridization expansion continuous time quantum Monte Carlo. Using the self-energy and the longitudinal static susceptibility, we obtain a phase diagram in the temperature-gap plane. The separatrix between the low-temperature local moment phase and the high temperature generalized Fermi liquid phase is shown to be the lower bound of the critical scaling region of the zero gap interacting quantum critical point. We have computed the nuclear magnetic spin-lattice relaxation rate, the Knight shift, and the Korringa ratio, which show strong deviations for any non-zero gap from the corresponding quantities in the gapless Kondo screened impurity case. This work is supported by NSF DMR-1237565 and NSF EPSCoR Cooperative Agreement EPS-1003897 with additional support from the Louisiana Board of Regents, and by CSIR and DST, India.
Demonstration of quantum logic gates in liquid crystal nuclear magnetic resonance
Marjanska, Malgorzata; Chuang, Isaac L.; Kubinec, Mark G.
2000-03-15
{sup 1}H-{sup 13}C heteronuclear dipolar couplings are used to produce the NMR (nuclear magnetic resonance) version of a two bit controlled-NOT quantum logic gate. This gate is coupled with the Hadamard gate to complete a circuit which generates the Einstein-Podolsky-Rosen (EPR) state which is the maximally entangled state of a pair of spins. The EPR state is crucial for the potential exponential speed advantage of quantum computers over their classical counterparts. We sample the deviation density matrix of the two spin system to verify the presence of the EPR state. EPR state lifetimes are also measured with this technique, thereby demonstrating the viability of liquid crystals as a platform for quantum computing. (c) 2000 American Institute of Physics.
Relaxation and coherent oscillations in the spin dynamics of II-VI diluted magnetic quantum wells
NASA Astrophysics Data System (ADS)
Ungar, F.; Cygorek, M.; Tamborenea, P. I.; Axt, V. M.
2015-10-01
We study theoretically the ultrafast spin dynamics of II-VI diluted magnetic quantum wells in the presence of spin-orbit interaction. We extend a recent study where it was shown that the spin-orbit interaction and the exchange sd coupling in bulk and quantum wells can compete resulting in qualitatively new dynamics when they act simultaneously. We concentrate on Hg1-x-yMnxCdyTe quantum wells, which have a highly tunable Rashba spin-orbit coupling. Our calculations use a recently developed formalism which incorporates electronic correlations originating from the exchange sd-coupling. We find that the dependence of electronic spin oscillations on the excess energy changes qualitatively depending on whether or not the spin-orbit interaction dominates or is of comparable strength with the sd interaction.
Kumar, D. Sanjeev Chatterjee, Ashok; Mukhopadhyay, Soma
2015-05-15
The magnetization of a parabolic quantum dot has been studied as a function of temperature and external magnetic field in the presence of Rashba, Dresselhaus Spin Orbit Interactions (SOI) and the electron-electron interactions. By the introduction of a simple and physically reasonable model potential, the problem has been solved exactly up to second order in both the SOI terms. Both the SOI found to be showing considerable effects on the magnetization of the quantum dot. The effect of electron-electron interaction on the magnetization also has been studied.
Magnetocaloric effect and magnetic cooling near a field-induced quantum-critical point
Wolf, Bernd; Tsui, Yeekin; Jaiswal-Nagar, Deepshikha; Tutsch, Ulrich; Honecker, Andreas; Remović-Langer, Katarina; Hofmann, Georg; Prokofiev, Andrey; Assmus, Wolf; Donath, Guido; Lang, Michael
2011-01-01
The presence of a quantum-critical point (QCP) can significantly affect the thermodynamic properties of a material at finite temperatures T. This is reflected, e.g., in the entropy landscape S(T,r) in the vicinity of a QCP, yielding particularly strong variations for varying the tuning parameter r such as pressure or magnetic field B. Here we report on the determination of the critical enhancement of ∂S/∂B near a B-induced QCP via absolute measurements of the magnetocaloric effect (MCE), (∂T/∂B)S and demonstrate that the accumulation of entropy around the QCP can be used for efficient low-temperature magnetic cooling. Our proof of principle is based on measurements and theoretical calculations of the MCE and the cooling performance for a Cu2+-containing coordination polymer, which is a very good realization of a spin-½ antiferromagnetic Heisenberg chain—one of the simplest quantum-critical systems.
Magnetic breakdown and Landau level spectra of a tunable double-quantum-well Fermi surface
Simmons, J.A.; Harff, N.E.; Lyo, S.K.; Klem, J.F.; Boebinger, G.S.; Pfeiffer, L.N.; West, K.W.
1997-12-31
By measuring longitudinal resistance, the authors map the Landau level spectra of double quantum wells as a function of both parallel (B{sub {parallel}}) and perpendicular (B{sub {perpendicular}}) magnetic fields. In this continuously tunable highly non-parabolic system, the cyclotron masses of the two Fermi surface orbits change in opposite directions with B{sub {parallel}}. This causes the two corresponding ladders of Landau levels formed at finite B{sub {perpendicular}} to exhibit multiple crossings. They also observe a third set of landau levels, independent of B{sub {parallel}}, which arise from magnetic breakdown of the Fermi surface. Both semiclassical and full quantum mechanical calculations show good agreement with the data.
NASA Astrophysics Data System (ADS)
Fu, Zhen-Guo; Zhang, Ping; Wang, Zhigang; Li, Shu-Shen
2012-04-01
We theoretically study the effect of localized magnetic impurities on two-dimensional topological superconductor (TSC). We show that the local density of states (LDOS) can be tuned by the effective exchange field m, the chemical potential μ of TSC, and the distance Δr as well as the relative spin angle α between two impurities. The changes in Δr between two impurities alter the interference and result in significant modifications to the bonding and antibonding states. Furthermore, the bound-state spin LDOS induced by single and double magnetic impurity scattering, the quantum corrals and the quantum mirages are also discussed. Finally, we briefly compare the impurities in TSC with those in topological insulators.
Quantum logic gates from time-dependent global magnetic field in a system with constant exchange
Nenashev, A. V. Dvurechenskii, A. V.; Zinovieva, A. F.; Gornov, A. Yu.; Zarodnyuk, T. S.
2015-03-21
We propose a method that implements a universal set of one- and two-quantum-bit gates for quantum computation in a system of coupled electron pairs with constant non-diagonal exchange interaction. In our proposal, suppression of the exchange interaction is performed by the continual repetition of single-spin rotations. A small g-factor difference between the electrons allows for addressing qubits and avoiding strong magnetic field pulses. Numerical experiments were performed to show that, to implement the one- and two-qubit operations, it is sufficient to change the strength of the magnetic field by a few Gauss. This introduces one and then the other electron in a resonance. To determine the evolution of the two-qubit system, we use the algorithms of optimal control theory.
Quantum magnetism without lattices in strongly interacting one-dimensional spinor gases
NASA Astrophysics Data System (ADS)
Deuretzbacher, F.; Becker, D.; Bjerlin, J.; Reimann, S. M.; Santos, L.
2014-07-01
We show that strongly interacting multicomponent gases in one dimension realize an effective spin chain, offering an alternative simple scenario for the study of one-dimensional (1D) quantum magnetism in cold gases in the absence of an optical lattice. The spin-chain model allows for an intuitive understanding of recent experiments and for a simple calculation of relevant observables. We analyze the adiabatic preparation of antiferromagnetic and ferromagnetic ground states, and show that many-body spin states may be efficiently probed in tunneling experiments. The spin-chain model is valid for more than two components, opening the possibility of realizing SU(N) quantum magnetism in strongly interacting 1D alkaline-earth-metal or ytterbium Fermi gases.
Single-spin measurements for quantum computation using magnetic resonance force microscopy
Berman, G. P.; Borgonovi, F.; Rinkevicius, Z.; Tsifrinovich, V. I.
2004-01-01
The quantum theory of a singlespin measurements using a magnetic resonance force microscopy is presented. We use an oscillating cantilever-driven adiabatic reversals technique. The frequency shift of the cantilever vibrations is estimated. We show that the frequency shift causes the formation of the Schroedinger cat state for the cantilever. The interaction between the cantilever and the environment quickly destroys the coherence between the two cantilever trajectories. It is shown that using partial adiabatic reversals one can obtain a significant increase in the frequency shift. We discuss the possibility of sub-magneton spin density detection in molecules using magnetic resonance force microscopy.
Magnetic field effect on the Coulomb interaction of acceptors in semimagnetic quantum dot
Kalpana, P.; Merwyn, A.; Nithiananthi, P.; Jayakumar, K.; Reuben, Jasper D.
2015-06-24
The Coulomb interaction of holes in a Semimagnetic Cd{sub 1-x}Mn{sub x}Te / CdTe Spherical and Cubical Quantum Dot (SMQD) in a magnetic field is studied using variational approach in the effective mass approximation. Since these holes in QD show a pronounced collective behavior, while distinct single particle phenomena is suppressed, their interaction in confined potential becomes very significant. It has been observed that acceptor-acceptor interaction is more in cubical QD than in spherical QD which can be controlled by the magnetic field. The results are presented and discussed.
Magnetic Flux Effect on a Kondo-Induced Electric Polarization in a Triangular Triple Quantum Dot
NASA Astrophysics Data System (ADS)
Koga, Mikito; Matsumoto, Masashige; Kusunose, Hiroaki
2014-08-01
A magnetic flux effect is studied theoretically on an electric polarization induced by the Kondo effect in a triangular triple-quantum-dot system, where one of the three dots is connected to a metallic lead. This electric polarization exhibits an Aharonov-Bohm oscillation as a function of the magnetic flux penetrating through the triangular loop. The numerical renormalization group analysis reveals how the oscillation pattern depends on the Kondo coupling of a local spin with lead electrons, which is sensitive to the point contact with the lead. It provides an experimental implication that the Kondo effect is the origin of the emergent electric polarization.
NASA Astrophysics Data System (ADS)
Koga, M.; Matsumoto, M.; Kusunose, H.
2015-03-01
The Kondo effect plays an important role in emergence of electric polarization in a triangular triple-quantum-dot system, where one of the three dots is point-contacted with a single lead, and a magnetic flux penetrates through the triangular loop. The Kondo-induced electric polarization exhibits an Aharonov-Bohm type oscillation as a function of the magnetic flux. Our theoretical study shows various oscillation patterns associated with the field-dependent mixing of twofold orbitally degenerate ground states and their sensitivity to the point contact.
Singh, Akhilesh K.; Barik, Puspendu; Ullrich, Bruno E-mail: bruno.ullrich@yahoo.com
2014-12-15
We observed changes of the transmitted monochromatic light passing through a colloidal PbS quantum dot film on glass owing to an applied moderate (smaller than 1 T) magnetic field under ambient conditions. The observed alterations show a square dependence on the magnetic field increase that cannot be achieved with bulk semiconductors. The findings point to so far not recognized application potentials of quantum dots.
NASA Astrophysics Data System (ADS)
Yamamoto, Daisuke; Marmorini, Giacomo; Danshita, Ippei
2015-01-01
Magnetization processes of spin-1 /2 layered triangular-lattice antiferromagnets (TLAFs) under a magnetic field H are studied by means of a numerical cluster mean-field method with a scaling scheme. We find that small antiferromagnetic couplings between the layers give rise to several types of extra quantum phase transitions among different high-field coplanar phases. Especially, a field-induced first-order transition is found to occur at H ≈0.7 Hs, where Hs is the saturation field, as another common quantum effect of ideal TLAFs in addition to the well-established one-third plateau. Our microscopic model calculation with appropriate parameters shows excellent agreement with experiments on Ba3CoSb2O9 [T. Susuki et al., Phys. Rev. Lett. 110, 267201 (2013)]. Given this fact, we suggest that the Co2 + -based compounds may allow for quantum simulations of intriguing properties of this simple frustrated model, such as quantum criticality and supersolid states.
Yamamoto, Daisuke; Marmorini, Giacomo; Danshita, Ippei
2015-01-16
Magnetization processes of spin-1/2 layered triangular-lattice antiferromagnets (TLAFs) under a magnetic field H are studied by means of a numerical cluster mean-field method with a scaling scheme. We find that small antiferromagnetic couplings between the layers give rise to several types of extra quantum phase transitions among different high-field coplanar phases. Especially, a field-induced first-order transition is found to occur at H≈0.7H_{s}, where H_{s} is the saturation field, as another common quantum effect of ideal TLAFs in addition to the well-established one-third plateau. Our microscopic model calculation with appropriate parameters shows excellent agreement with experiments on Ba_{3}CoSb_{2}O_{9} [T. Susuki et al., Phys. Rev. Lett. 110, 267201 (2013)]. Given this fact, we suggest that the Co^{2+}-based compounds may allow for quantum simulations of intriguing properties of this simple frustrated model, such as quantum criticality and supersolid states. PMID:25635561
Space-charge waves in magnetized and collisional quantum plasma columns confined in carbon nanotubes
Bagheri, Mehran; Abdikian, Alireza
2014-04-15
We study the dispersion relation of electrostatic waves propagating in a column of quantum magnetized collisional plasma embraced completely by a metallic single-walled carbon nanotubes. The analysis is based on the quantum linearized hydrodynamic formalism of collective excitations within the quasi-static approximation. It is shown when the electronic de Broglie's wavelength of the plasma is comparable in the order of magnitude to the radius of the nanotube, the quantum effects are quite meaningful and our model anticipates one acoustical and two optical space-charge waves which are positioned into three propagating bands. With increasing the nanotube radius, the features of the acoustical branch remain unchanged, yet two distinct optical branches are degenerated and the classical behavior is recovered. This study might provide a platform to create new finite transverse cross section quantum magnetized plasmas and to devise nanometer dusty plasmas based on the metallic carbon nanotubes in the absence of either a drift or a thermal electronic velocity and their existence could be experimentally examined.
Triple-quantum-filtered sodium magnetic resonance imaging
NASA Astrophysics Data System (ADS)
Hancu, Ileana
2001-11-01
In this thesis, a method to selectively detect sodium ions in slow motion, the triple-quantum (TQ) filtering technique, was implemented for the first time in a whole- body, clinical MR scanner. The method was used for collecting images from in vivo normal and neoplastic human brain tissues, and cartilage tissue. It was confirmed that the TQ filter rejects signals from liquid-like environments, and it became apparent that this method might become useful for the diagnosis and prognosis of brain neoplasms. Additional issues related to implementing a TQ filter in clinical scanners were considered. The effect of B1 and B0 imperfections was analyzed for the three- and four-pulse TQ filters. It was concluded that the signal loss due to B1 inhomogeneities in the four-pulse filter could be overwhelmingly high if flip angles are not perfect. The three-pulse filter leads to much smaller signal losses, and has the advantage that signal biases can be corrected for by post-processing. The effect of relaxation during the application of RF pulses was also considered. Since pulse-widths normally used for hard 90-degree pulses in clinical scanners are comparable to the relaxation times of sodium ions, the amount of TQ-filtered signal loss due to this effect was checked, theoretically and experimentally. By increasing the pulse width of the hard 90-degree RF pulses from 100μs to 500μs in a cartilage sample, about 15% of the TQ-signal is lost, therefore shorter pulses will not dramatically increase the TQ-filtered signal strength. A new method to selectively detect sodium ions in anisotropic environments was also developed. Following the application of a hard 90-degree pulse, quadrupolar polarization is created during the application of a spin- lock (SL) field only in the presence of residual quadrupolar couplings (if B1 is on the same order of magnitude with these couplings). This coherence is then converted into observable signal by a coherence- transfer pulse. The SL-filter has
Quantum tunneling of two coupled single-molecular magnets
NASA Astrophysics Data System (ADS)
Hu, Jianming; Chen, Zhide; Shen, Shunqing
2003-03-01
Jian-Ming Hu, Zhi-De Chen and Shun-Qing Shen Department of Physics, The University of Hong Kong Pokfulam Road, Hong Kong December 02, 2002 Very recently a supramolecular dimer of two single-molecule magnets (SMM) was reported to be synthesized successfully. Two single-molecule magnets are coupled antiferromagnetically to form a supramolecule dimer. We study the coupling effect and tunneling process by the numerical exact diagonalization method. The sweeping rate effect in the derivatives of hysteresis loops has been quantitatively investigated using the modified Landau-Zener model. In addiction we find that exchange coupling between the two SMMs provides a biased field to expel the tunneling between SMMs to two new resonant points via an intermediate state, and direct tunneling is prohibited. The model parameters are calculated for the dimer based on the tunneling process. The outcome indicates that the coupling effect will not change the parameters of each SMM too much at all. This work is supported by a CRCG grant of The University of Hong Kong.
Out of equilibrium energy dynamics in low dimensional quantum magnets
NASA Astrophysics Data System (ADS)
Langer, Stephan; Heyl, Markus; McCulloch, Ian; Heidrich-Meisner, Fabian
2012-02-01
We investigate the real-time dynamics of the energy density in spin-1/2 XXZ chains using two types of quenches resulting in initial states which feature an inhomogeneous distribution of local energies [1]. The first involves quenching bonds in the center of the chain from antiferromagnetic to ferromagnetic exchange interactions. The second quench involves an inhomogeneous magnetic field, inducing both, an inhomogeneous magnetization profile [2] and local energy density. The simulations are carried out using the adaptive time-dependent density matrix renormalization group algorithm. We analyze the time-dependence of the spatial variance of the bond energies and the local energy currents which both yield necessary criteria for ballistic or diffusive energy dynamics. For both setups, our results are consistent with ballistic behavior, both in the massless and the massive phase. For the massless regime, we compare our numerical results to bosonization and the non-interacting limit finding very good agreement. The velocity of the energy wave-packets can be understood as the average velocity of excitations induced by the quench. [4pt] [1] Langer et al. Phys. Rev. B in press; arXiv:1107.4136[0pt] [2] Langer et al. Phys. Rev. B 79, 214409 (2009)
Quantum speed limit for a relativistic electron in a uniform magnetic field
NASA Astrophysics Data System (ADS)
Villamizar, D. V.; Duzzioni, E. I.
2015-10-01
We analyze the influence of relativistic effects on the minimum evolution time between two orthogonal states of a quantum system. Defining the initial state as a homogeneous superposition between two Hamiltonian eigenstates of an electron in a uniform magnetic field, we obtain a relation between the minimum evolution time and the displacement of the mean radial position of the electron wave packet. The quantum speed limit time is calculated for an electron dynamics described by Dirac and Schrödinger-Pauli equations considering different parameters, such as the strength of magnetic field and the linear momentum of the electron in the axial direction. We highlight that when the electron undergoes a region with extremely strong magnetic field the relativistic and nonrelativistic dynamics differ substantially, so that the description given by the Schrödinger-Pauli equation enables the electron to travel faster than c , which is prohibited by Einstein's theory of relativity. This approach allows a connection between the abstract Hilbert space and the space-time coordinates, besides the identification of the most appropriate quantum dynamics used to describe the electron motion.
Numerical Study of Spin-Dependent Transport Through a Magnetic Quantum Wire with Lattice Vacancy
NASA Astrophysics Data System (ADS)
Jafari, A.; Ghoranneviss, M.
2016-03-01
The impact of lattice vacancy on the spin dependent transport properties of a magnetic-quantum wire (MQW) has been investigated. A simple tight binding Hamiltonian to describe the model is used, where the quantum wire is attached to two semi-infinite one-dimensional non-magnetic electrodes. Based on the Landauer-Buttiker formalism all the calculations are performed numerically which describe two-terminal conductance. The results suggest that in presence of vacancy the transmission reduces and vacancy creates quasilocalized states around zero energy (E f = 0). In order to investigate spin-filtering effect of (MQW), the degree of polarization in the presence and absences of vacancy has been studied. Also it is found that the effect of vacancy decreases when the size of MQW increases. The results show that a magnetic quantum wire can be used as a spin filter. The application of the predicted results may be useful in designing molecular spin-polarized transistors in the future.
A quantum description of radiation damping and the free induction signal in magnetic resonance
Tropp, James
2013-07-07
We apply the methods of cavity quantum electrodynamics (CQED), to obtain a microscopic and fully quantum-mechanical picture of radiation damping in magnetic resonance, and the nascent formation of the free induction signal. Numerical solution of the Tavis-Cummings model - i.e., multiple spins 1/2 coupled to a lossless single-mode cavity - shows in fine detail the transfer of Zeeman energy, via spin coherence, to excite the cavity - represented here by a quantized LC resonator. The case of a single spin is also solved analytically. Although the motion of the Bloch vector is non-classical, we nonetheless show that the quantum mechanical Rabi nutation frequency (as enhanced by cavity coupling and stimulated emission) gives realistic estimates of macroscopic signal strength and the radiation damping constant in nuclear magnetic resonance. We also show how to introduce dissipation: cavity losses by means of a master equation, and relaxation by the phenomenological method of Bloch. The failure to obtain the full Bloch equations (unless semi-classical conditions are imposed on the cavity) is discussed in light of similar issues arising in CQED (and in earlier work in magnetic resonance as well), as are certain problems relative to quantization of the electromagnetic near-field.
Magnetic-Field-Assisted Terahertz Quantum Cascade Laser Operating up to 225 K
NASA Technical Reports Server (NTRS)
Wade, A.; Fedorov, G.; Smirnov, D.; Kumar, S.; Williams, B. S.; Hu, Q.; Reno, J. L.
2008-01-01
Advances in semiconductor bandgap engineering have resulted in the recent development of the terahertz quantum cascade laser1. These compact optoelectronic devices now operate in the frequency range 1.2-5 THz, although cryogenic cooling is still required2.3. Further progress towards the realization of devices operating at higher temperatures and emitting at longer wavelengths (sub-terahertz quantum cascade lasers) is difficult because it requires maintaining a population inversion between closely spaced electronic sub-bands (1 THz approx. equals 4 meV). Here, we demonstrate a magnetic-field-assisted quantum cascade laser based on the resonant-phonon design. By applying appropriate electrical bias and strong magnetic fields above 16 T, it is possible to achieve laser emission from a single device over a wide range of frequencies (0.68-3.33 THz). Owing to the suppression of inter-landau-level non-radiative scattering, the device shows magnetic field assisted laser action at 1 THz at temperatures up to 215 K, and 3 THz lasing up to 225 K.
NASA Astrophysics Data System (ADS)
Abdullah, Nzar Rauf; Tang, Chi-Shung; Manolescu, Andrei; Gudmundsson, Vidar
2016-09-01
We investigate theoretically the balance of the static magnetic and the dynamical photon forces in the electron transport through a quantum dot in a photon cavity with a single photon mode. The quantum dot system is connected to external leads and the total system is exposed to a static perpendicular magnetic field. We explore the transport characteristics through the system by tuning the ratio, \\hslash {ωγ}/\\hslash {ωc} , between the photon energy, \\hslash {ωγ} , and the cyclotron energy, \\hslash {ωc} . Enhancement in the electron transport with increasing electron–photon coupling is observed when \\hslash {ωγ}/\\hslash {ωc}>1 . In this case the photon field dominates and stretches the electron charge distribution in the quantum dot, extending it towards the contact area for the leads. Suppression in the electron transport is found when \\hslash {ωγ}/\\hslash {ωc}<1 , as the external magnetic field causes circular confinement of the charge density around the dot.
Wavefunction dynamics in a quantum-dot electron pump under a high magnetic field
NASA Astrophysics Data System (ADS)
Ryu, Sungguen; Kataoka, Masaya; Sim, Heung-Sun
2015-03-01
A quantum-dot electron pump, formed and operated by applying time-dependent potential barriers to a two dimensional electron gas system, provides a promising redefinition of ampere. The pump operation consists of capturing an electron from a reservoir into a quantum dot and ejecting it to another reservoir. The capturing process has been theoretically understood by a semi-classical treatment of the tunneling between the dot and reservoir. But the dynamics of the wavefunction of the captured electron in the ejection process has not been theoretically addressed, although it is useful for enhancing pump accuracy and for utilizing the pump as a single-electron source for mesoscopic quantum electron devices. We study the dynamics under a strong magnetic field that leads to magnetic confinement of the captured electron, which dominates over the electrostatic confinement of the dot. We find that the wave packet of the captured electron has the Gaussian form with the width determined by the strength of the magnetic field, and that the time evolution of the packet follows the classical drift motion, with maintaining the Gaussian form. We discuss the possible signatures of the wave packet dynamics in experiments.
Optically pumped nuclear magnetic resonance in the quantum Hall regimes
NASA Astrophysics Data System (ADS)
Barrett, S. E.; Dabbagh, G.; Pfeiffer, L. N.; West, K. W.; Tycko, R.
1996-11-01
We review our recent measurements of the Knight shift 0268-1242/11/11S/005/img1 and spin-lattice relaxation time 0268-1242/11/11S/005/img2 of the 0268-1242/11/11S/005/img3 nuclei located in n-doped GaAs quantum wells using optically pumped NMR, for Landau level filling 0268-1242/11/11S/005/img4 and temperature 0268-1242/11/11S/005/img5. 0268-1242/11/11S/005/img6 (0268-1242/11/11S/005/img7 the electron spin polarization 0268-1242/11/11S/005/img8) drops precipitously on either side of 0268-1242/11/11S/005/img9, which is evidence that the charged excitations of the 0268-1242/11/11S/005/img9 ground state are finite-size skyrmions. For 0268-1242/11/11S/005/img11, the data are consistent with a many-body ground state which is not fully spin polarized, with a very small spin excitation gap that increases as 0268-1242/11/11S/005/img12.
Terahertz excitations near the quantum critical point in the 1D Ising chain quantum magnet CoNb2O6
NASA Astrophysics Data System (ADS)
Morris, Christopher M.; Valdés Aguilar, R.; Koopayeh, S.; McQueen, T. M.; Armitage, N. P.
2013-03-01
The one-dimensional magnet CoNb2O6 was recently demonstrated to be an excellent realization of a one-dimensional quantum Ising spin chain. It has been shown to undergo a quantum phase transition in a magnetic field oriented transverse to its ferromagnetically aligned spin chains. Low energy spin-flip excitations in the chains were recently observed via inelastic neutron scattering.[2] The energy spectrum of these excitations was shown to have a interesting energy scaling governed by symmetries of the E8 exceptional Lie group. Here, time-domain terahertz spectroscopy (TDTS) is used to investigate these optically active spin flip excitations in CoNb2O6 in an external magnetic field. For static magnetic fields oriented transverse to the spin chains, the terahertz excitations show evidence of the phase transitions that occur near the quantum critical magnetic field. Additional spin flip excitations are also observed for longitudinally oriented magnetic fields. Work supported by The Institute of Quantum Matter under DOE grant DE-FG02-08ER46544 and by the Gordon and Betty Moore Foundation.
High-field ESR studies of the quantum spin magnet CaCu2O3
NASA Astrophysics Data System (ADS)
Goiran, M.; Costes, M.; Broto, J. M.; Chou, F. C.; Klingeler, R.; Arushanov, E.; Drechsler, S.-L.; Büchner, B.; Kataev, V.
2006-05-01
We report an electron spin resonance (ESR) study of the s = 1/2 Heisenberg pseudo-ladder magnet CaCu2O3 in pulsed magnetic fields up to 40 T. At sub-terahertz frequencies we observe an ESR signal originating from a small amount of uncompensated spins residing presumably at the imperfections of the strongly antiferromagnetically correlated host spin lattice. The data give evidence that these few per cent of 'extra' spin states are coupled strongly to the bulk spins and are involved in the antiferromagnetic (AF) ordering at TN = 25 K. By mapping the frequency/resonance field diagram we have determined a small gap for magnetic excitations below TN of the order of ~0.3 0.8 meV. Such a small value of the gap explains the occurrence of the spin-flop transition in CaCu2O3 at weak magnetic fields μ0Hsf ~ 3 T. Qualitative changes of the ESR response with the increasing field strength give indications that strong magnetic fields reduce the AF correlations and may even suppress the long-range magnetic order in CaCu2O3. ESR data support scenarios with a significant role of the 'extra' spin states for the properties of low-dimensional quantum magnets.
NASA Astrophysics Data System (ADS)
Avetisyan, Siranush; Chakraborty, Tapash; Pietiläinen, Pekka
2016-07-01
Magnetization of anisotropic quantum dots in the presence of the Rashba spin-orbit interaction has been studied for three and four interacting electrons in the dot for non-zero values of the applied magnetic field. We observe unique behaviors of magnetization that are direct reflections of the anisotropy and the spin-orbit interaction parameters independently or concurrently. In particular, there are saw-tooth structures in the magnetic field dependence of the magnetization, as caused by the electron-electron interaction, that are strongly modified in the presence of large anisotropy and high strength of the spin-orbit interactions. We also report the temperature dependence of magnetization that indicates the temperature beyond which these structures due to the interactions disappear. Additionally, we found the emergence of a weak sawtooth structure in magnetization for three electrons in the high anisotropy and large spin-orbit interaction limit that was explained as a result of merging of two low-energy curves when the level spacings evolve with increasing values of the anisotropy and the spin-orbit interaction strength.
Salim, Michael A; Willow, Soohaeng Yoo; Hirata, So
2016-05-28
Ice Ih displays several anomalous thermodynamic properties such as thermal contraction at low temperatures, an anomalous volume isotope effect (VIE) rendering the volume of D2O ice greater than that of H2O ice, and a pressure-induced transition to the high-density amorphous (HDA) phase. Furthermore, the anomalous VIE increases with temperature, despite its quantum-mechanical origin. Here, embedded-fragment ab initio second-order many-body perturbation (MP2) theory in the quasiharmonic approximation (QHA) is applied to the Gibbs energy of an infinite, proton-disordered crystal of ice Ih at wide ranges of temperatures and pressures. The quantum effect of nuclei moving in anharmonic potentials is taken into account from first principles without any empirical or nonsystematic approximation to either the electronic or vibrational Hamiltonian. MP2 predicts quantitatively correctly the thermal contraction at low temperatures, which is confirmed to originate from the volume-contracting hydrogen-bond bending modes (acoustic phonons). It qualitatively reproduces (but underestimates) the thermal expansion at higher temperatures, caused by the volume-expanding hydrogen-bond stretching (and to a lesser extent librational) modes. The anomalous VIE is found to be the result of subtle cancellations among closely competing isotope effects on volume from all modes. Consequently, even ab initio MP2 with the aug-cc-pVDZ and aug-cc-pVTZ basis sets has difficulty reproducing this anomaly, yielding qualitatively varied predictions of the sign of the VIE depending on such computational details as the choice of the embedding field. However, the temperature growth of the anomalous VIE is reproduced robustly and is ascribed to the librational modes. These solid-state MP2 calculations, as well as MP2 Born-Oppenheimer molecular dynamics, find a volume collapse and a loss of symmetry and long-range order in ice Ih upon pressure loading of 2.35 GPa or higher. Concomitantly, rapid softening of
NASA Astrophysics Data System (ADS)
Salim, Michael A.; Willow, Soohaeng Yoo; Hirata, So
2016-05-01
Ice Ih displays several anomalous thermodynamic properties such as thermal contraction at low temperatures, an anomalous volume isotope effect (VIE) rendering the volume of D2O ice greater than that of H2O ice, and a pressure-induced transition to the high-density amorphous (HDA) phase. Furthermore, the anomalous VIE increases with temperature, despite its quantum-mechanical origin. Here, embedded-fragment ab initio second-order many-body perturbation (MP2) theory in the quasiharmonic approximation (QHA) is applied to the Gibbs energy of an infinite, proton-disordered crystal of ice Ih at wide ranges of temperatures and pressures. The quantum effect of nuclei moving in anharmonic potentials is taken into account from first principles without any empirical or nonsystematic approximation to either the electronic or vibrational Hamiltonian. MP2 predicts quantitatively correctly the thermal contraction at low temperatures, which is confirmed to originate from the volume-contracting hydrogen-bond bending modes (acoustic phonons). It qualitatively reproduces (but underestimates) the thermal expansion at higher temperatures, caused by the volume-expanding hydrogen-bond stretching (and to a lesser extent librational) modes. The anomalous VIE is found to be the result of subtle cancellations among closely competing isotope effects on volume from all modes. Consequently, even ab initio MP2 with the aug-cc-pVDZ and aug-cc-pVTZ basis sets has difficulty reproducing this anomaly, yielding qualitatively varied predictions of the sign of the VIE depending on such computational details as the choice of the embedding field. However, the temperature growth of the anomalous VIE is reproduced robustly and is ascribed to the librational modes. These solid-state MP2 calculations, as well as MP2 Born-Oppenheimer molecular dynamics, find a volume collapse and a loss of symmetry and long-range order in ice Ih upon pressure loading of 2.35 GPa or higher. Concomitantly, rapid softening of
NASA Astrophysics Data System (ADS)
Pixley, Jedediah H.
Rare earth and actinide metal compounds have emerged as quintessential systems to experimentally and theoretically explore zero temperature quantum phase transitions. These so called heavy fermion metals provide a platform to systematically study physics on the edge of our understanding, where conventional approaches fail to describe the experimental observations. In this thesis, we are concerned with the theoretical description of the different types of quantum phases and phase transitions that are possible within heavy fermion metals. We first focus on understanding the unconventional quantum critical scaling properties observed in heavy fermion metals. Guided by the extended dynamical mean field theory (EDMFT) of the Kondo lattice, we study the physics of Kondo destruction in simplified quantum impurity models. Using the continuous time quantum Monte Carlo (CT-QMC), we show Kondo destroyed quantum critical points (QCPs) give rise to local correlation functions that obey frequency and magnetic field over temperature scaling, and have a linear in temperature relaxation rate. Our results are consistent with the experiments on the quantum critical heavy fermion metals YbRh2Si2, CeCu6- xAux, and beta-YbAlB4. Motivated by experiments on CeRhIn5 and related heavy fermion systems, we then focus on the superconducting properties of the Kondo destroyed QCPs. We introduce and solve an effective model that has both Kondo destruction and pairing correlations, using a combination of CTQMC and the numerical renormalization group (NRG) methods. We then solve the cluster EDMFT equations across the QCP for two and three dimensional magnetic fluctuations, using the CT-QMC as the cluster solver. In the two dimensional case, we find that the Kondo screening is driven critical at the antiferromagnetic QCP. In each case studied, we find that the pairing susceptibility is strongly enhanced in the vicinity of the QCP. Our results point to the exciting possibility of an unconventional
Bose glass and Mott glass of quasiparticles in a doped quantum magnet.
Yu, Rong; Yin, Liang; Sullivan, Neil S; Xia, J S; Huan, Chao; Paduan-Filho, Armando; Oliveira, Nei F; Haas, Stephan; Steppke, Alexander; Miclea, Corneliu F; Weickert, Franziska; Movshovich, Roman; Mun, Eun-Deok; Scott, Brian L; Zapf, Vivien S; Roscilde, Tommaso
2012-09-20
The low-temperature states of bosonic fluids exhibit fundamental quantum effects at the macroscopic scale: the best-known examples are Bose-Einstein condensation and superfluidity, which have been tested experimentally in a variety of different systems. When bosons interact, disorder can destroy condensation, leading to a 'Bose glass'. This phase has been very elusive in experiments owing to the absence of any broken symmetry and to the simultaneous absence of a finite energy gap in the spectrum. Here we report the observation of a Bose glass of field-induced magnetic quasiparticles in a doped quantum magnet (bromine-doped dichloro-tetrakis-thiourea-nickel, DTN). The physics of DTN in a magnetic field is equivalent to that of a lattice gas of bosons in the grand canonical ensemble; bromine doping introduces disorder into the hopping and interaction strength of the bosons, leading to their localization into a Bose glass down to zero field, where it becomes an incompressible Mott glass. The transition from the Bose glass (corresponding to a gapless spin liquid) to the Bose-Einstein condensate (corresponding to a magnetically ordered phase) is marked by a universal exponent that governs the scaling of the critical temperature with the applied field, in excellent agreement with theoretical predictions. Our study represents a quantitative experimental account of the universal features of disordered bosons in the grand canonical ensemble. PMID:22996552
NASA Astrophysics Data System (ADS)
Kim, Jeongwoo; Jhi, Seung-Hoon; Wu, Ruqian
Realization of transverse electric currents without external magnetic fields, so called the quantum anomalous Hall effect (QAHE), is achieved in Cr-doped topological insulating (Bi,Sb)2Te3 compounds. However, detailed mechanism of QAHE and magnetic ordering in topological insulators (TIs) is still unclear with several models in controversy. We study the origin of QAHE in magnetic impurity-doped TIs using first-principles calculations. We investigate a possibility of the quantum anomalous Hall phase in conventional three-dimensional topological insulators, such as Bi2Se3, Bi2Te3, and Sb2Te3. We find that Sb2Te3 is the most suitable compound for realizing QAHE, because it maintains insulating phase and relatively strong ferromagnetic ordering in a wide range of Cr doping while Bi2Se3 and Bi2Te3 become metallic even by a small amount of Cr doping. Contrary to previous predictions, the kinetic exchange is responsible for the magnetic phase of Cr-doped TIs and it induces spin-polarized valence and conduction bands in Sb2Te3. We also discuss the role of Bi doping in topological surfaces states of Cr-doped Sb2Te3, which leads to QAHE in (Bi,Sb)2Te3. Work was supported as part of the SHINES, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. SC0012670.
Vinante, A. Falferi, P.; Mezzena, R.
2014-10-15
Superconducting Quantum Interference Device (SQUID) microsusceptometers have been widely used to study magnetic properties of materials at microscale. As intrinsically balanced devices, they could also be exploited for direct SQUID-detection of nuclear magnetic resonance (NMR) from micron sized samples, or for SQUID readout of mechanically detected NMR from submicron sized samples. Here, we demonstrate a double balancing technique that enables achievement of very low residual imbalance of a SQUID microsusceptometer over a wide bandwidth. In particular, we can generate ac magnetic fields within the SQUID loop as large as 1 mT, for frequencies ranging from dc up to a few MHz. As an application, we demonstrate direct detection of NMR from {sup 1}H spins in a glycerol droplet placed directly on top of the 20 μm SQUID loops.
Magnetic-field control of quantum critical points of valence transition.
Watanabe, Shinji; Tsuruta, Atsushi; Miyake, Kazumasa; Flouquet, Jacques
2008-06-13
We study the mechanism of how critical end points of first-order valence transitions are controlled by a magnetic field. We show that the critical temperature is suppressed to be a quantum critical point (QCP) by a magnetic field, and unexpectedly, the QCP exhibits nonmonotonic field dependence in the ground-state phase diagram, giving rise to the emergence of metamagnetism even in the intermediate valence-crossover regime. The driving force of the field-induced QCP is clarified to be cooperative phenomena of the Zeeman and Kondo effects, which create a distinct energy scale from the Kondo temperature. This mechanism explains the peculiar magnetic response in CeIrIn(5) and the metamagnetic transition in YbXCu(4) for X=In as well as the sharp contrast between X=Ag and Cd. PMID:18643524
Kondo-type transport through a quantum dot under magnetic fields
Dong, Bing; Lei, X. L.
2001-06-15
In this paper, we investigate the Kondo correlation effects on linear and nonlinear transport in a quantum dot connected to reservoirs under finite magnetic fields, using the slave-boson mean field approach suggested by Kotliar and Ruckenstein [Phys. Rev. Lett. >57, 1362 (1986)]. A brief comparison between the present formulation and other slave-boson formulation is presented to justify this approach. The numerical results show that the linear conductance near electron-hole symmetry is suppressed by the application of the magnetic fields, but an anomalous enhancement is predicted in the nonsymmetry regime. The effect of external magnetic fields on the nonlinear differential conductances is discussed for the Kondo system. A significant reduction of the peak splitting is observed due to the strong Kondo correlation, which agrees well with experimental data.
Magnetic field control of the intraband optical absorption in two-dimensional quantum rings
Olendski, O.; Barakat, T.
2014-02-28
Linear and nonlinear optical absorption coefficients of the two-dimensional semiconductor ring in the perpendicular magnetic field B are calculated within independent electron approximation. Characteristic feature of the energy spectrum are crossings of the levels with adjacent nonpositive magnetic quantum numbers as the intensity B changes. It is shown that the absorption coefficient of the associated optical transition is drastically decreased at the fields corresponding to the crossing. Proposed model of the Volcano disc allows to get simple mathematical analytical results, which provide clear physical interpretation. An interplay between positive linear and intensity-dependent negative cubic absorption coefficients is discussed; in particular, critical light intensity at which additional resonances appear in the total absorption dependence on the light frequency is calculated as a function of the magnetic field and levels' broadening.
Violation of Bell’s inequality in a spin 1/2 quantum magnet
Chakraborty, Tanmoy Singh, Harkirat Mitra, Chiranjib
2014-04-24
Violation of Bell’s inequality test has been established as an efficient tool to determine the presence of entanglement in quantum spin 1/2 magnets. Herein, macroscopic thermodynamic quantities, namely, magnetic susceptibility and specific heat have been employed to perform Bell’s inequality test for [NH{sub 4}CuPO{sub 4}, H{sub 2}O], a spin 1/2 antiferromagnet with nearest neighbor interactions. The mean value of the Bell operator is quantified and plotted as a function of temperature. The threshold temperature is determined above which the Bell’s inequality is not violated and a good consistency is found between the analyses done on magnetic and thermal data.
Quantum capacitance of an ultrathin topological insulator film in a magnetic field
Tahir, M.; Sabeeh, K.; Schwingenschlögl, U.
2013-01-01
We present a theoretical study of the quantum magnetocapacitance of an ultrathin topological insulator film in an external magnetic field. The study is undertaken to investigate the interplay of the Zeeman interaction with the hybridization between the upper and lower surfaces of the thin film. Determining the density of states, we find that the electron-hole symmetry is broken when the Zeeman and hybridization energies are varied relative to each other. This leads to a change in the character of the magnetocapacitance at the charge neutrality point. We further show that in the presence of both Zeeman interaction and hybridization the magnetocapacitance exhibits beating at low and splitting of the Shubnikov de Haas oscillations at high perpendicular magnetic field. In addition, we address the crossover from perpendicular to parallel magnetic field and find consistency with recent experimental data. PMID:23405275
Strain and localization effects in InGaAs(N) quantum wells: Tuning the magnetic response
Lopes-Oliveira, V. Herval, L. K. S.; Orsi Gordo, V.; Cesar, D. F.; Godoy, M. P. F. de; Galvão Gobato, Y.; Henini, M.; Khatab, A.; Sadeghi, M.; Wang, S.; Schmidbauer, M.
2014-12-21
We investigated effects of localization and strain on the optical and magneto-optical properties of diluted nitrogen III–V quantum wells theoretically and experimentally. High-resolution x-ray diffraction, photoluminescence (PL), and magneto-PL measurements under high magnetic fields up to 15 T were performed at low temperatures. Bir-Pikus Hamiltonian formalism was used to study the influence of strain, confinement, and localization effects. The circularly polarized magneto-PL was interpreted considering localization aspects in the valence band ground state. An anomalous behavior of the electron-hole pair magnetic shift was observed at low magnetic fields, ascribed to the increase in the exciton reduced mass due to the negative effective mass of the valence band ground state.
Engineering quantum magnetism in one-dimensional trapped Fermi gases with p -wave interactions
NASA Astrophysics Data System (ADS)
Yang, Lijun; Guan, Xiwen; Cui, Xiaoling
2016-05-01
The highly controllable ultracold atoms in a one-dimensional (1D) trap provide a new platform for the ultimate simulation of quantum magnetism. In this regard, the Néel antiferromagnetism and the itinerant ferromagnetism are of central importance and great interest. Here we show that these magnetic orders can be achieved in the strongly interacting spin-1/2 trapped Fermi gases with additional p -wave interactions. In this strong-coupling limit, the 1D trapped Fermi gas exhibits an effective Heisenberg spin X X Z chain in the anisotropic p -wave scattering channels. For a particular p -wave attraction or repulsion within the same species of fermionic atoms, the system displays ferromagnetic domains with full spin segregation or the antiferromagnetic spin configuration in the ground state. Such engineered magnetisms are likely to be probed in a quasi-1D trapped Fermi gas of 40K atoms with very close s -wave and p -wave Feshbach resonances.
Nature of Pressure-induced Insulating States in Simple Metals
NASA Astrophysics Data System (ADS)
Naumov, Ivan; Hemley, Russell
As experimentally established, all the alkali metals and heavy alkaline earth metals (Ca, Sr and Ba) become progressively less conductive on compression, at least up to some critical limit over a broad pressure range. Of these metals, Li and Na clearly undergo pressure-induced metal-insulator transitions, which may also be called reverse Mott transitions. Here, using group theory arguments and first-principles calculations, we show that such transitions can be understood in terms of band representations introduced by Zak. The valence bands in the insulating states are described by simple and composite band representations constructed from localized Wannier functions centered on points unoccupied by atoms. The character of the Wannier functions is closely related to the degree of s-p(-d) hybridization and reflects multi-center chemical bonding in these insulating states. The conditions under which an insulating state is allowed for structures having an integer number of atoms per primitive unit cell as well as re-entrant (i.e., metal-insulator-metal) transition sequences are detailed, resulting in predictions of semimetallic phases with flat surface states. The general principles developed are tested and applied to the alkali and alkaline earth metals, including elements where high-pressure insulating phases have been identified or reported (e.g., Li, Na, and Ca). This research was supported by EFree, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award DESC0001057.
High-pressure-induced water penetration into 3-isopropylmalate dehydrogenase
Nagae, Takayuki; Kawamura, Takashi; Chavas, Leonard M. G.; Niwa, Ken; Hasegawa, Masashi; Kato, Chiaki; Watanabe, Nobuhisa
2012-03-01
Structures of 3-isopropylmalate dehydrogenase were determined at pressures ranging from 0.1 to 650 MPa. Comparison of these structures gives a detailed picture of the swelling of a cavity at the dimer interface and the generation of a new cleft on the molecular surface, which are accompanied by water penetration. Hydrostatic pressure induces structural changes in proteins, including denaturation, the mechanism of which has been attributed to water penetration into the protein interior. In this study, structures of 3-isopropylmalate dehydrogenase (IPMDH) from Shewanella oneidensis MR-1 were determined at about 2 Å resolution under pressures ranging from 0.1 to 650 MPa using a diamond anvil cell (DAC). Although most of the protein cavities are monotonically compressed as the pressure increases, the volume of one particular cavity at the dimer interface increases at pressures over 340 MPa. In parallel with this volume increase, water penetration into the cavity could be observed at pressures over 410 MPa. In addition, the generation of a new cleft on the molecular surface accompanied by water penetration could also be observed at pressures over 580 MPa. These water-penetration phenomena are considered to be initial steps in the pressure-denaturation process of IPMDH.
Transdermal deferoxamine prevents pressure-induced diabetic ulcers
Duscher, Dominik; Neofytou, Evgenios; Wong, Victor W.; Maan, Zeshaan N.; Rennert, Robert C.; Januszyk, Michael; Rodrigues, Melanie; Malkovskiy, Andrey V.; Whitmore, Arnetha J.; Galvez, Michael G.; Whittam, Alexander J.; Brownlee, Michael; Rajadas, Jayakumar; Gurtner, Geoffrey C.
2015-01-01
There is a high mortality in patients with diabetes and severe pressure ulcers. For example, chronic pressure sores of the heels often lead to limb loss in diabetic patients. A major factor underlying this is reduced neovascularization caused by impaired activity of the transcription factor hypoxia inducible factor-1 alpha (HIF-1α). In diabetes, HIF-1α function is compromised by a high glucose-induced and reactive oxygen species-mediated modification of its coactivator p300, leading to impaired HIF-1α transactivation. We examined whether local enhancement of HIF-1α activity would improve diabetic wound healing and minimize the severity of diabetic ulcers. To improve HIF-1α activity we designed a transdermal drug delivery system (TDDS) containing the FDA-approved small molecule deferoxamine (DFO), an iron chelator that increases HIF-1α transactivation in diabetes by preventing iron-catalyzed reactive oxygen stress. Applying this TDDS to a pressure-induced ulcer model in diabetic mice, we found that transdermal delivery of DFO significantly improved wound healing. Unexpectedly, prophylactic application of this transdermal delivery system also prevented diabetic ulcer formation. DFO-treated wounds demonstrated increased collagen density, improved neovascularization, and reduction of free radical formation, leading to decreased cell death. These findings suggest that transdermal delivery of DFO provides a targeted means to both prevent ulcer formation and accelerate diabetic wound healing with the potential for rapid clinical translation. PMID:25535360
Pressure-induced phase transitions and metallization in VO2
NASA Astrophysics Data System (ADS)
Bai, Ligang; Li, Quan; Corr, Serena A.; Meng, Yue; Park, Changyong; Sinogeikin, Stanislav V.; Ko, Changhyun; Wu, Junqiao; Shen, Guoyin
2015-03-01
We report the results of pressure-induced phase transitions and metallization in VO2 based on synchrotron x-ray diffraction, electrical resistivity, and Raman spectroscopy. Our isothermal compression experiments at room temperature and 383 K show that the room temperature monoclinic phase (M 1 ,P 21/c ) and the high-temperature rutile phase (R ,P 42/m n m ) of VO2 undergo phase transitions to a distorted M 1 monoclinic phase (M 1' ,P 21/c ) above 13.0 GPa and to an orthorhombic phase (CaCl2-like, P n n m ) above 13.7 GPa, respectively. Upon further compression, both high-pressure phases transform into a new phase (phase X ) above 34.3 and 38.3 GPa at room temperature and 383 K, respectively. The room temperature M 1 -M 1' phase transition structurally resembles the R -CaCl2 phase transition at 383 K, suggesting a second-order displacive type of transition. Contrary to previous studies, our electrical resistivity results, Raman measurements, as well as ab initio calculations indicate that the new phase X , rather than the M 1' phase, is responsible for the metallization under pressure. The metallization mechanism is discussed based on the proposed crystal structure.
Pressure induced reactions amongst calcium aluminate hydrate phases
Moon, Ju-hyuk; Oh, Jae Eun; Balonis, Magdalena; Glasser, Fredrik P.; Clark, Simon M.; Monteiro, Paulo J.M.
2011-06-15
The compressibilities of two AFm phases (straetlingite and calcium hemicarboaluminate hydrate) and hydrogarnet were obtained up to 5 GPa by using synchrotron high-pressure X-ray powder diffraction with a diamond anvil cell. The AFm phases show abrupt volume contraction regardless of the molecular size of the pressure-transmitting media. This volume discontinuity could be associated to a structural transition or to the movement of the weakly bound interlayer water molecules in the AFm structure. The experimental results seem to indicate that the pressure-induced dehydration is the dominant mechanism especially with hygroscopic pressure medium. The Birch-Murnaghan equation of state was used to compute the bulk modulus of the minerals. Due to the discontinuity in the pressure-volume diagram, a two stage bulk modulus of each AFm phase was calculated. The abnormal volume compressibility for the AFm phases caused a significant change to their bulk modulus. The reliability of this experiment is verified by comparing the bulk modulus of hydrogarnet with previous studies.
Long-distance super-exchange and quantum magnetic relaxation in a hybrid metal-organic framework
NASA Astrophysics Data System (ADS)
Ying, Tian; Shipeng, Shen; Junzhuang, Cong; Liqin, Yan; Yisheng, Chai; Young, Sun
2016-01-01
The hybrid metal-organic framework [(CH3)2NH2]Fe(HCOO)3 with a perovskite-like structure exhibits a variety of unusual magnetic behaviors at low temperatures. While the long-distance super-exchange through the Fe-O-CH-O-Fe exchange path leads to a canted antiferromagnetic ordering at TN ˜ 19 K, a second transition of magnetic blocking develops at TB ˜ 9 K. The stair-shaped magnetization hysteresis loops below TB resemble the behaviors of resonant quantum tunneling of magnetization in single-molecular quantum magnets. Moreover, the magnetic relaxation also exhibits several features of resonant quantum relaxation, such as the exponential law with a single characteristic relaxation time, and the nonmonotonic dependence of relaxation rate on the applied magnetic field with a much faster relaxation around the resonant fields. The origin of quantum tunneling behaviors in the [(CH3)2NH2]Fe(HCOO)3 metal-organic framework is discussed in terms of magnetic phase separation due to the modification of hydrogen bonding on the long-distance super-exchange interaction. Project supported by the National Natural Science Foundation of China (Grant Nos. 11227405, 51371192, and 51371193) and the Chinese Academy of Sciences (Grant No. XDB07030200).
Quantum tricks with femtosecond light pulses teach magnetic devices to think ultrafast
NASA Astrophysics Data System (ADS)
Perakis, I. E.; Lingos, P. C.; Wang, J.
2014-03-01
The technological demand to push the gigahertz switching speed limit of today's magnetic memory/logic devices into the terahertz (1THz=1ps-1) regime underlies the entire field of spin-electronics and integrated multi- functional devices. This challenge is met by all-optical magnetic switching based on coherent spin manipulation By analogy to femto-chemistry and photosynthetic dynamics where photo-products of chemical/biochemical re- actions can be influenced by creating suitable superpositions of molecular states, femtosecond (fs) laser-excited coherence between spin/orbital/charge states can switch magnetic orders, by "suddenly" breaking the delicate balance between competing phases of correlated materials, e.g., the colossal magneto-resistive (CMR) manganites suitable for applications. Here we discuss femtosecond (fs) all-optical switching from antiferro- to ferromagnetic ordering via establishment of a magnetization increase within ˜100 fs, while the laser field still interacts with the system. Such non-equilibrium ferromagnetic correlations arise from quantum spin-flip fluctuations corre- lated with coherent superpositions of electronic states. The development of ferromagnetic correlations during the fs laser pulse reveals an initial quantum coherent regime of magnetism, clearly distinguished from the pi- cosecond lattice-heating regime characterized by phase separation. We summarize a microscopic theory based on density matrix equations of motion for composite fermion Hubbard operators, instead of bare electrons, that take into account the strong spin and charge local correlations. Our work merges two fields, femto-magnetism in metals/band insulators and non-equilibrium phase transitions of strongly correlated electrons, where local interactions exceeding the kinetic energy produce a complex balance of competing orders.
Femtosecond switching of magnetism via strongly correlated spin-charge quantum excitations.
Li, Tianqi; Patz, Aaron; Mouchliadis, Leonidas; Yan, Jiaqiang; Lograsso, Thomas A; Perakis, Ilias E; Wang, Jigang
2013-04-01
The technological demand to push the gigahertz (10(9) hertz) switching speed limit of today's magnetic memory and logic devices into the terahertz (10(12) hertz) regime underlies the entire field of spin-electronics and integrated multi-functional devices. This challenge is met by all-optical magnetic switching based on coherent spin manipulation. By analogy to femtosecond chemistry and photosynthetic dynamics--in which photoproducts of chemical and biochemical reactions can be influenced by creating suitable superpositions of molecular states--femtosecond-laser-excited coherence between electronic states can switch magnetic order by 'suddenly' breaking the delicate balance between competing phases of correlated materials: for example, manganites exhibiting colossal magneto-resistance suitable for applications. Here we show femtosecond (10(-15) seconds) photo-induced switching from antiferromagnetic to ferromagnetic ordering in Pr0.7Ca0.3MnO3, by observing the establishment (within about 120 femtoseconds) of a huge temperature-dependent magnetization with photo-excitation threshold behaviour absent in the optical reflectivity. The development of ferromagnetic correlations during the femtosecond laser pulse reveals an initial quantum coherent regime of magnetism, distinguished from the picosecond (10(-12) seconds) lattice-heating regime characterized by phase separation without threshold behaviour. Our simulations reproduce the nonlinear femtosecond spin generation and underpin fast quantum spin-flip fluctuations correlated with coherent superpositions of electronic states to initiate local ferromagnetic correlations. These results merge two fields, femtosecond magnetism in metals and band insulators, and non-equilibrium phase transitions of strongly correlated electrons, in which local interactions exceeding the kinetic energy produce a complex balance of competing orders. PMID:23552945
NASA Astrophysics Data System (ADS)
Pelliccione, Matthew; Jenkins, Alec; Ovartchaiyapong, Preeti; Reetz, Christopher; Emmanouilidou, Eve; Ni, Ni; Bleszynski Jayich, Ania C.
2016-08-01
High-spatial-resolution magnetic imaging has driven important developments in fields ranging from materials science to biology. However, to uncover finer details approaching the nanoscale with greater sensitivity requires the development of a radically new sensor technology. The nitrogen–vacancy (NV) defect in diamond has emerged as a promising candidate for such a sensor on the basis of its atomic size and quantum-limited sensing capabilities. It has remained an outstanding challenge to implement the NV centre as a nanoscale scanning magnetic probe at cryogenic temperatures, however, where many solid-state systems exhibit non-trivial magnetic order. Here, we present NV magnetic imaging down to 6 K with 3 μT Hz–1/2 field sensitivity, and use the technique to image vortices in the iron pnictide superconductor BaFe2(As0.7P0.3)2 with critical temperature Tc = 30 K. The expansion of NV-based magnetic imaging to cryogenic temperatures will enable future studies of previously inaccessible nanoscale magnetism in condensed-matter systems.
The effect of current-induced spin switching in the presence of quantum tunneling of magnetization
NASA Astrophysics Data System (ADS)
Misiorny, Maciej; Barnaś, Józef
2013-03-01
Knowledge of transport properties of individual large-spin (S > 1 / 2) atoms/molecules exhibiting magnetic anisotropy is of key importance from the point of view of information processing technologies. The ultimate aim is to incorporate such objects as functional elements of spintronic devices, with the objective of employing spin-polarized currents to control the magnetic state of the system. In particular, for an atom/molecule with the predominant `easy-axis' uniaxial magnetic anisotropy this allows for switching the system's spin between two metastable states. However, the uniaxial component of magnetic anisotropy, underlying the magnetic bistability, is frequently accompanied by the transverse one, whose presence manifests, e.g., as quantum tunneling of magnetization (QTM). Here, we show that not only does QTM induce an effective energy barrier for the spin switching, but also its effect on the transport reveals as an additional signal in transport characteristics. Furthermore, we propose how to experimentally investigate QTM by means of the STM inelastic transport spectroscopy. also at Adam Mickiewicz University
Pelliccione, Matthew; Jenkins, Alec; Ovartchaiyapong, Preeti; Reetz, Christopher; Emmanouilidou, Eve; Ni, Ni; Bleszynski Jayich, Ania C
2016-08-01
High-spatial-resolution magnetic imaging has driven important developments in fields ranging from materials science to biology. However, to uncover finer details approaching the nanoscale with greater sensitivity requires the development of a radically new sensor technology. The nitrogen-vacancy (NV) defect in diamond has emerged as a promising candidate for such a sensor on the basis of its atomic size and quantum-limited sensing capabilities. It has remained an outstanding challenge to implement the NV centre as a nanoscale scanning magnetic probe at cryogenic temperatures, however, where many solid-state systems exhibit non-trivial magnetic order. Here, we present NV magnetic imaging down to 6 K with 3 μT Hz(-1/2) field sensitivity, and use the technique to image vortices in the iron pnictide superconductor BaFe2(As0.7P0.3)2 with critical temperature Tc = 30 K. The expansion of NV-based magnetic imaging to cryogenic temperatures will enable future studies of previously inaccessible nanoscale magnetism in condensed-matter systems. PMID:27136130
NASA Astrophysics Data System (ADS)
Boda, Aalu; Chatterjee, Ashok
2016-09-01
The problem of a neutral hydrogenic donor (D0) centre located at the centre of a GaAs quantum dot with Gaussian confinement is studied in the presence of an external magnetic field. The ground and the first excited state energies and the corresponding binding energies are obtained as functions of the potential strength, quantum dot radius and the magnetic field using a variational method. It is suggested that the first excited state of the D0 centre is bound for sufficiently strong confinement potential. The 1 s - 2p- transition energy and the magnetic susceptibilities for the ground and the first excited states are also determined.
Effect of disorder on the pressure-induced superconducting state of CeAu 2Si 2
NASA Astrophysics Data System (ADS)
Ren, Z.; Giriat, G.; Scheerer, G. W.; Lapertot, G.; Jaccard, D.
2015-03-01
CeAu2Si2 is a newly discovered pressure-induced heavy fermion superconductor, which shows very unusual interplay between superconductivity and magnetism under pressure. Here we compare the results of high-pressure measurements on single-crystalline CeAu2Si2 samples with different levels of disorder. It is found that while the magnetic properties are essentially sample independent, superconductivity is rapidly suppressed when the residual resistivity of the sample increases. We show that the depression of bulk Tc can be well understood in terms of pair breaking by nonmagnetic disorder, which strongly suggests an unconventional pairing state in pressurized CeAu2Si2 . Furthermore, increasing the level of disorder leads to the emergence of another phase transition at T* within the magnetic phase, which might be in competition with superconductivity.
Quantum criticality and inhomogeneous magnetic order in Fe-doped α -YbAlB4
NASA Astrophysics Data System (ADS)
MacLaughlin, D. E.; Kuga, K.; Shu, Lei; Bernal, O. O.; Ho, P.-C.; Nakatsuji, S.; Huang, K.; Ding, Z. F.; Tan, C.; Zhang, Jian
2016-06-01
The intermediate-valent polymorphs α - and β -YbAlB4 exhibit quantum criticality and other novel properties not usually associated with intermediate valence. Iron doping induces quantum criticality in α -YbAlB4 and magnetic order in both compounds. We report results of muon spin relaxation (μ SR ) experiments in α -YbAl1 -xFexB4 , x =0.014 and 0.25. For x =0.014 we find no evidence for magnetic order down to 25 mK. The dynamic muon spin relaxation rate λd exhibits a power-law temperature dependence λd∝T-a , a =0.40 (4 ) , in the temperature range 100 mK-2 K, in disagreement with predictions by theories of antiferromagnetic (AFM) or valence quantum critical behavior. For x =0.25 , where AFM order develops in the temperature range 7.5-10 K, we find coexistence of meso- or macroscopically segregated paramagnetic and AFM phases, with considerable disorder in the latter down to 2 K.
Magnetic Field Tuning and Quantum Interference in a Cooper Pair Splitter
NASA Astrophysics Data System (ADS)
Fülöp, G.; Domínguez, F.; d'Hollosy, S.; Baumgartner, A.; Makk, P.; Madsen, M. H.; Guzenko, V. A.; Nygârd, J.; Schönenberger, C.; Levy Yeyati, A.; Csonka, S.
2015-11-01
Cooper pair splitting (CPS) is a process in which the electrons of the naturally occurring spin-singlet pairs in a superconductor are spatially separated using two quantum dots. Here, we investigate the evolution of the conductance correlations in an InAs CPS device in the presence of an external magnetic field. In our experiments the gate dependence of the signal that depends on both quantum dots continuously evolves from a slightly asymmetric Lorentzian to a strongly asymmetric Fano-type resonance with increasing field. These experiments can be understood in a simple three-site model, which shows that the nonlocal CPS leads to symmetric line shapes, while the local transport processes can exhibit an asymmetric shape due to quantum interference. These findings demonstrate that the electrons from a Cooper pair splitter can propagate coherently after their emission from the superconductor and how a magnetic field can be used to optimize the performance of a CPS device. In addition, the model calculations suggest that the estimate of the CPS efficiency in the experiments is a lower bound for the actual efficiency.
Parallel magnetic field-induced conductance fluctuations in GaAs/AlGaAs ballistic quantum dots.
NASA Astrophysics Data System (ADS)
Faniel, S.; Gustin, C.; Melinte, S.; Hackens, B.; Bayot, V.; Shayegan, M.
2004-03-01
We present magnetotransport measurements in ballistic quantum dots under a parallel magnetic field. The dots were fabricated on two different GaAs/AlGaAs quantum wells with thicknesses of 15 and and 45 nm and with one and two subbands occupied, respectively. The samples were patterned using e-beam lithography and wet etching. A Cr/Au electrostatic top gate was used in order to tune the width of the dot openings. The measurements were performed down to 300 mK with the magnetic field applied strictly parallel to the plane of the two-dimensional electron gas. For both dots, we observe universal conductance fluctuations and, in the case of the wide quantum well, a reduction of their amplitude at large magnetic field. We discuss these conductance fluctuations in terms of orbital effect(V.I. Fal'ko and T. Jungwirth, Phys Rev B 65), 081306 (2002) and magnetic subband depopulation.
Energy Gap Dependence on Mn Content in a Diluted Magnetic Quantum Dot
NASA Astrophysics Data System (ADS)
Nalini, P.; John Peter, A.
2011-04-01
Positively charged donor exciton binding energy is computed as a function of quantum-dot size within the single band effective mass approximation for different Mn contents in Cd1-xinMnxin Te/Cd1-xoutMnxout Te. The exciton bound polaron is computed for 0 <= x <= 0.08, on the Mn mole fraction. We determine the energy gap using the mean field approximation and incorporate the exchange interaction between the carrier and the magnetic impurity. The interband emission energy is studied with the height and radius of the cylindrical quantum dot. Valence-band anisotropy is included in our theoretical model using different hole masses in different spatial directions. Spin polaronic shifts as functions of quantum-dot radius and Mn concentration are estimated using the mean field theory. It is found that (i) the energy gap depends on the Mn mole fraction, (ii) it increases linearly with an increase in Mn content, and (iii) the effect is more pronounced for a narrow dot, showing the quantum size effects. Our results are in good agreement with other recently published reports.
NASA Astrophysics Data System (ADS)
Gustin, C.; Faniel, S.; Hackens, B.; Melinte, S.; Shayegan, M.; Bayot, V.
2005-04-01
Using two-dimensional electron gases (2DEGs) confined to wide and narrow quantum wells, we study the magnetoconductance of ballistic quantum dots as a function of the well width and the tilt angle of the magnetic field B with respect to the 2DEG. Both the wide and narrow quantum well dots feature magnetoconductance fluctuations (MCFs) at intermediate tilt angles, due to the finite thickness of the electron layer and the field-induced orbital effect. As B approaches a strictly parallel configuration, a saturation of the MCFs’ spectral distribution is observed, combined with the persistence of a limited number of frequency components in the case of the narrow quantum well dot. It is found that the onset of saturation strongly depends on the width of the confining well. Using the results of self-consistent Poisson-Schrödinger simulations, the magnetoconductance is rescaled as a function of the Fermi level in the 2DEG. We perform a power spectrum analysis of the parallel field-induced MCFs in the energy space and find a good agreement with theoretical predictions.
NASA Astrophysics Data System (ADS)
Mejri, Youssef
2016-06-01
In this article, we study the boundary inverse problem of determining the aligned magnetic field appearing in the magnetic Schrödinger equation in a periodic quantum cylindrical waveguide, by knowledge of the Dirichlet-to-Neumann map. We prove a Hölder stability estimate with respect to the Dirichlet-to-Neumann map, by means of the geometrical optics solutions of the magnetic Schrödinger equation.
Conventional versus unconventional magnetic polarons: ZnMnTe/ZnSe and ZnTe/ZnMnSe quantum dots
NASA Astrophysics Data System (ADS)
Barman, B.; Tsai, Y.; Scrace, T.; Murphy, J. R.; Cartwright, A. N.; Pientka, J. M.; Zutic, I.; McCombe, B. D.; Petrou, A.; Sellers, I. R.; Oszwaldowski, R.; Petukhov, A.; Fan, W. C.; Chou, W. C.; Yang, C. S.
2014-08-01
We used time resolved photoluminescence (TRPL) spectroscopy to compare the properties of magnetic polarons in two related, spatially indirect, II-VI epitaxially grown quantum dot systems. In sample A (ZnMnTe/ZnSe), the photoexcited holes are confined in the magnetic ZnMnTe quantum dots (QDs), while the electrons remain in the surrounding non-magnetic ZnSe matrix. In sample B (ZnTe/ZnMnSe) on the other hand, the holes are confined in the non-magnetic ZnTe QDs and the electrons move in the magnetic ZnMnSe matrix. The magnetic polaron formation energies, EMP , in these samples were measured from the temporal red-shift of the excitonic emission peak. The magnetic polarons in the two samples exhibit distinct characteristics. In sample A, the magnetic polaron is strongly bound with EMP=35 meV. Furthermore, EMP has unconventionally weak dependence of on both temperature T and magnetic field Bappl . In contrast, magnetic polarons in sample B show conventional characteristics with EMP decreasing with increasing temperature and increasing external magnetic field. We attribute the difference in magnetic polaron properties between the two types of QDs to the difference in the location of the Mn ions in the respective structures.
Quantum phase transitions in triangular lattice Heisenberg anti-ferromagnet in a magnetic field
NASA Astrophysics Data System (ADS)
Ye, Mengxing; Chubukov, Andrey
We present the zero temperature phase diagram of a large S Heisenberg anti-ferromagnet on a frustrated triangular lattice with the nearest neighbor (J1) and the next nearest neighbor (J2) interactions, in a magnetic field. We show that the classical model has an ``accidental'' degeneracy for all J2 /J1 and all fields below the saturation field, which gives rise to the extended manifold of the ground state spin configurations. Quantum fluctuations, however, lift this degeneracy. For small J2 /J1 , they select one of three different co-planar states, depending on the field value. We argue that above some critical ratio of J2 /J1 , which weakly depends on a magnetic field, these fluctuations select the stripe phase. We analyze in detail the mechanism of the selection of the stripe phase and explore the nature of the quantum phase transition in a magnetic field between the ordered phases as J2 /J1 passes through a critical value.
Scattering-induced quantum correlation in electronic waveguides with static magnetic impurities
NASA Astrophysics Data System (ADS)
Ghanbari-Adivi, E.; Soltani, M.; Alami, Z.; Sheikhali, M.
2016-07-01
Entanglement generation due to low-energy scattering of the transporting electrons in an electronic waveguide by a quantum dot magnetic impurity is theoretically investigated. The transverse confining potential of the waveguide is considered as a two-dimensional harmonic potential, and the interaction of the electron with the impurity is described by a zero-range pseudopotential modulated by an Ising or a Heisenberg spin interaction. Our calculation shows that the scattering process leads to creation of a considerable amount of entanglement in the state of the reflected and transmitted electrons. The situation is extended to the scattering of the electrons by two well-separated magnetic impurities localized on the nanowire axis. It is shown that the scattering process causes the magnetic impurities embedded in the nanowire to share their quantum information; subsequently, they can be entangled by spin interaction with the injected electron. The created entanglement between the impurities is calculated and discussed. It is shown that the exact three-dimensional problem can be approximated as a one-dimensional problem under certain circumstances. The approximate results are compared to exact calculations and discussed.
Magnetic field-induced control of transport in multiterminal focusing quantum billiards
NASA Astrophysics Data System (ADS)
Morfonios, C.; Buchholz, D.; Schmelcher, P.
2011-05-01
By exploring the four-terminal transmission of a semielliptic open quantum billiard in dependence of its geometry and an applied magnetic field, it is shown that a controllable switching of currents between the four terminals can be obtained. Depending on the eccentricity of the semiellipse and the width and placement of the leads, high transmittivity at zero magnetic field is reached either through states guided along the curved boundary or focused onto the straight boundary of the billiard. For small eccentricity, attachment of leads at the ellipse foci can yield optimized corresponding transmission, while departures from this behavior demonstrate the inapplicability of solely classical considerations in the deep quantum regime. The geometrically determined transmission is altered by the phase-modulating and deflecting effect of the magnetic field, which switches the pairs of leads connected by high transmittivity. It is shown that the elliptic boundary is responsible for these very special transport properties. At higher field strengths edge states form and the multiterminal transmission coefficients are determined by the topology of the billiard. The combination of magnetotransport with geometrically optimized transmission behavior leads to an efficient control of the current through the multiterminal structure.
Thermal Quantum Discord in Pure Dzyaloshinskii—Moriya Model with Magnetic Field
NASA Astrophysics Data System (ADS)
Li, Da-Chuang; Li, Xiao-Man; Cao, Zhuo-Liang
2016-06-01
We investigate the effects of the directions of Dzyaloshinskii—Moriya (DM) interaction vector and magnetic field on the quantum discord in the pure DM model. For different directions of DM vector, we find that there are different optimal parameter components of magnetic field. Moreover, we find that the optimal parameter components rules are the same for the Hamiltonian H1 and H2. According to the rules, for a certain axial DM vector, we can get the maximal quantum discord by adjusting the direction of the external magnetic field, which is feasible under the current experimental technology. Supported by the National Natural Science Foundation of China under Grant Nos. 11204061, 11374085, 11104057, and 11204002, the Anhui Provincial Natural Science Foundation under Grant No. 1408085MA16, the Anhui Provincial Candidates for Academic and Technical Leaders Foundation under Grant No. 2015H052, the discipline top-notch talents Foundation and the Excellent Young Talents Support Plan of Anhui Provincial Universities. Ming Yang is supported by National Natural Science Foundation of China under Grant No. 11274010, the Specialized Research Fund for the Doctoral Program of Higher Education under Grant No. 20113401110002, the 211 Project of Anhui University, and the Personnel Department of Anhui Province
AC transport in p-Ge/GeSi quantum well in high magnetic fields
Drichko, I. L.; Malysh, V. A.; Smirnov, I. Yu.; Golub, L. E.; Tarasenko, S. A.; Suslov, A. V.; Mironov, O. A.; Kummer, M.; Känel, H. von
2014-08-20
The contactless surface acoustic wave technique is implemented to probe the high-frequency conductivity of a high-mobility p-Ge/GeSi quantum well structure in the regime of integer quantum Hall effect (IQHE) at temperatures 0.3–5.8 K and magnetic fields up to 18 T. It is shown that, in the IQHE regime at the minima of conductivity, holes are localized and ac conductivity is of hopping nature and can be described within the “two-site” model. The analysis of the temperature and magnetic-field-orientation dependence of the ac conductivity at odd filing factors enables us to determine the effective hole g-factor, |g{sub zz}|≈4.5. It is shown that the in-plane component of the magnetic field leads to a decrease in the g-factor as well as increase in the cyclotron mass, which is explained by orbital effects in the complex valence band of germanium.
Trion X+ in vertically coupled type II quantum dots in threading magnetic field.
Horta-Piñeres, Sindi; Escorcia-Salas, Gene Elizabeth; Mikhailov, Ilia D; Sierra-Ortega, José
2012-01-01
We analyze the energy spectrum of a positively charged exciton confined in a semiconductor heterostructure formed by two vertically coupled, axially symmetrical type II quantum dots located close to each other. The electron in the structure is mainly located inside the dots, while the holes generally move in the exterior region close to the symmetry axis. The solutions of the Schrödinger equation are obtained by a variational separation of variables in the adiabatic limit. Numerical results are shown for bonding and anti-bonding lowest-lying of the trion states corresponding to the different quantum dots morphologies, dimensions, separation between them, thicknesses of the wetting layers, and the magnetic field strength. PMID:23013605
Magnetoresistance quantum oscillations in a magnetic two-dimensional electron gas
NASA Astrophysics Data System (ADS)
Kunc, J.; Piot, B. A.; Maude, D. K.; Potemski, M.; Grill, R.; Betthausen, C.; Weiss, D.; Kolkovsky, V.; Karczewski, G.; Wojtowicz, T.
2015-08-01
Magnetotransport measurements of Shubnikov-de Haas (SdH) oscillations have been performed on two-dimensional electron gases (2DEGs) confined in CdTe and CdMnTe quantum wells. The quantum oscillations in CdMnTe, where the 2DEG interacts with magnetic Mn ions, can be described by incorporating the electron-Mn exchange interaction into the traditional Lifshitz-Kosevich formalism. The modified spin splitting leads to characteristic beating pattern in the SdH oscillations, the study of which indicates the formation of Mn clusters resulting in direct anti-ferromagnetic Mn-Mn interaction. The Landau-level broadening in this system shows a peculiar decrease with increasing temperature, which could be related to statistical fluctuations of the Mn concentration.
Quantum magnetic flux lines, BPS vortex zero modes, and one-loop string tension shifts
NASA Astrophysics Data System (ADS)
Alonso-Izquierdo, A.; Mateos Guilarte, J.; de la Torre Mayado, M.
2016-08-01
Spectral heat kernel/zeta function regularization procedures are employed in this paper to control the divergences arising from vacuum fluctuations of Bogomolnyi-Prasad-Sommerfield vortices in the Abelian Higgs model. Zero modes of vortex fluctuations are the source of difficulties appearing when the standard Gilkey-de Witt expansion is the tool used in the calculations of one-loop shifts of vortex masses and string tensions. A modified GdW expansion is developed to diminish the impact of the infrared divergences due to the vortex zero modes of fluctuation. With this new technique at our disposal we compute the one-loop vortex mass shifts in the planar AHM and the quantum corrections to the string tension of the magnetic flux tubes living in three dimensions. In both cases it is observed that weak repulsive forces surge between these classically noninteracting topological defects caused by vacuum quantum fluctuations.
NASA Astrophysics Data System (ADS)
Zhao, Hong-Kang; Wang, Jian
2004-03-01
We have investigated the coherent mesoscopic transport through a quantum-dot (QD) embedded carbon nanotube ring (CNR) by employing the nonequilibrium Green's function (NGF) technique. The Landauer-Büttiker-like formula is presented to calculate the differential conductance and current-voltage characteristics. Due to the interference of the electrons transporting in the two paths of CNR, the resultant conductivity of electron through the system is determined by the compound concrete structure of CNR-QD system. The tunneling current appears quantum behavior obviously in the small region of source-drain bias. The conductance is adjusted by the gate voltage Vg and the magnetic flux φ. The reversal resonance has been displayed versus the gate voltage, and it is symmetric about Vg for the type I CNR, but it is asymmetric for the type II CNR. The phase inverse oscillations are also presented for the different types of CNRs.
Klich, I.; Lee, S.-H.; Iida, K.
2014-01-01
When spins are arranged in a lattice of triangular motif, the phenomenon of frustration leads to numerous energetically equivalent ground states, and results in exotic states such as spin liquid and spin ice. Here we report an alternative situation: a system, classically a liquid, freezes in the clean limit into a glassy state induced by quantum fluctuations. We call such glassy state a spin jam. The case in point is a frustrated magnet, where spins are arranged in a triangular network of bipyramids. Quantum corrections break the classical degeneracy into a set of aperiodic spin configurations forming local minima in a rugged energy landscape. This is established by mapping the problem into tiling with hexagonal tiles. The number of tessellations scales with the boundary length rather than its volume, showing the absence of local zero-energy modes. Low-temperature thermodynamics is discussed to compare it with other glassy materials. PMID:24686398
Magnetic field dependence of energy levels in biased bilayer graphene quantum dots
NASA Astrophysics Data System (ADS)
da Costa, D. R.; Zarenia, M.; Chaves, Andrey; Farias, G. A.; Peeters, F. M.
2016-02-01
Using the tight-binding approach, we study the influence of a perpendicular magnetic field on the energy levels of hexagonal, triangular, and circular bilayer graphene (BLG) quantum dots (QDs) with zigzag and armchair edges. We obtain the energy levels for AB (Bernal)-stacked BLG QDs in both the absence and the presence of a perpendicular electric field (i.e., biased BLG QDs). We find different regions in the spectrum of biased QDs with respect to the crossing point between the lowest-electron and -hole Landau levels of a biased BLG sheet. Those different regions correspond to electron states that are localized at the center, edge, or corner of the BLG QD. Quantum Hall corner states are found to be absent in circular BLG QDs. The spatial symmetry of the carrier density distribution is related to the symmetry of the confinement potential, the position of zigzag edges, and the presence or absence of interlayer inversion symmetry.
Kaiju, H. Kasa, H.; Mori, S.; Misawa, T.; Abe, T.; Nishii, J.; Komine, T.
2015-05-07
We investigate the Co thickness dependence of the structural and magnetic properties of Co thin-film electrodes sandwiched between borate glasses in spin quantum cross (SQC) devices that utilize stray magnetic fields. We also calculate the Co thickness dependence of the stray field between the two edges of Co thin-film electrodes in SQC devices using micromagnetic simulation. The surface roughness of Co thin films with a thickness of less than 20 nm on borate glasses is shown to be as small as 0.18 nm, at the same scanning scale as the Co film thickness, and the squareness of the hysteresis loop is shown to be as large as 0.96–1.0. As a result of the establishment of polishing techniques for Co thin-film electrodes sandwiched between borate glasses, we successfully demonstrate the formation of smooth Co edges and the generation of stray magnetic fields from Co edges. Theoretical calculation reveals that a strong stray field beyond 6 kOe is generated when the Co thickness is greater than 10 nm at a junction gap distance of 5 nm. From these experimental and calculation results, it can be concluded that SQC devices with a Co thickness of 10–20 nm can be expected to function as spin-filter devices.
Pressure-induced referred pain is expanded by persistent soreness.
Doménech-García, V; Palsson, T S; Herrero, P; Graven-Nielsen, T
2016-05-01
Several chronic pain conditions are accompanied with enlarged referred pain areas. This study investigated a novel method for assessing referred pain. In 20 healthy subjects, pressure pain thresholds (PPTs) were recorded and pressure stimuli (120% PPT) were applied bilaterally for 5 and 60 seconds at the infraspinatus muscle to induce local and referred pain. Moreover, PPTs were measured bilaterally at the shoulder, neck, and leg before, during, and after hypertonic saline-induced referred pain in the dominant infraspinatus muscle. The pressure and saline-induced pain areas were assessed on drawings. Subsequently, delayed onset muscle soreness was induced using eccentric exercise of the dominant infraspinatus muscle. The day-1 assessments were repeated the following day (day 2). Suprathreshold pressure stimulations and saline injections into the infraspinatus muscle caused referred pain to the frontal aspect of the shoulder/arm in all subjects. The 60-second pressure stimulation caused larger referred pain areas compared with the 5-second stimulation (P < 0.01). Compared with pressure stimulation, the saline-induced referred pain area was larger (P < 0.02). After saline-induced pain, the PPTs at the infraspinatus and supraspinatus muscles were reduced (P < 0.05), and the 5-second pressure-induced referred pain area was larger than baseline. Pressure pain thresholds at the infraspinatus and supraspinatus muscles were reduced at day 2 in the delayed onset muscle soreness side (P < 0.05). Compared with day 1, larger pressure and saline-induced referred pain areas were observed on day 2 (P < 0.05). Referred pain to the shoulder/arm was consistently induced and enlarged after 1 day of muscle soreness, indicating that the referred pain area may be a sensitive biomarker for sensitization of the pain system. PMID:26808146
NASA Astrophysics Data System (ADS)
Çakır, Bekir; Atav, Ülfet; Yakar, Yusuf; Özmen, Ayhan
2016-08-01
In this study we report a detailed theoretical investigation of the effect of an external magnetic field on the 1s-, 2p-, 3d- and 4f-energy states of a spherical quantum dot. We treat the contribution of the diamagnetic term as a perturbation and discuss the effect of the diamagnetic term on the 1s-, 2p-, 3d- and 4f-energy states. We also have calculated the Zeeman transition energies between 2p → 1s and 3d → 2p states with m = 0, ±1 and 0, ±1, ±2 as a function of dot radius and the magnetic field strength. The results show that the magnetic field, impurity charge and dot radius have a strong influence on the energy states and the Zeeman transitions. It is found that the energies of the electronic states with m < 0 addition of the diamagnetic term firstly decrease toward a minimum, and then increase with the increasing magnetic field strength. We have seen that as magnetic field intensity is adjusted, frequency of the emitted light can be changed for Zeeman transitions.
Dos Santos, Leonardo H R; Lanza, Arianna; Barton, Alyssa M; Brambleby, Jamie; Blackmore, William J A; Goddard, Paul A; Xiao, Fan; Williams, Robert C; Lancaster, Tom; Pratt, Francis L; Blundell, Stephen J; Singleton, John; Manson, Jamie L; Macchi, Piero
2016-02-24
The accurate electron density distribution and magnetic properties of two metal-organic polymeric magnets, the quasi-one-dimensional (1D) Cu(pyz)(NO3)2 and the quasi-two-dimensional (2D) [Cu(pyz)2(NO3)]NO3·H2O, have been investigated by high-resolution single-crystal X-ray diffraction and density functional theory calculations on the whole periodic systems and on selected fragments. Topological analyses, based on quantum theory of atoms in molecules, enabled the characterization of possible magnetic exchange pathways and the establishment of relationships between the electron (charge and spin) densities and the exchange-coupling constants. In both compounds, the experimentally observed antiferromagnetic coupling can be quantitatively explained by the Cu-Cu superexchange pathway mediated by the pyrazine bridging ligands, via a σ-type interaction. From topological analyses of experimental charge-density data, we show for the first time that the pyrazine tilt angle does not play a role in determining the strength of the magnetic interaction. Taken in combination with molecular orbital analysis and spin density calculations, we find a synergistic relationship between spin delocalization and spin polarization mechanisms and that both determine the bulk magnetic behavior of these Cu(II)-pyz coordination polymers. PMID:26811927
Pressure-induced change of the electronic state in the tetragonal phase of CaFe2As2
NASA Astrophysics Data System (ADS)
Sakaguchi, Yui; Ikeda, Shugo; Kuse, Tetsuji; Kobayashi, Hisao
2014-07-01
We have investigated the electronic states of single-crystal CaFe2As2 under hydrostatic pressure using 57Fe Mössbauer spectroscopy and magnetization measurements. The center shift and the quadrupole splitting were refined from observed 57Fe Mössbauer spectra using the single-crystalline sample under pressure at room temperature. A discontinuous decrease in the pressure dependence of the refined center shift was observed at 0.33 GPa without any anomaly in the pressure dependence of the refined quadrupole splitting, indicating a purely electronic state change in CaFe2As2 with a tetragonal structure. Such a change is shown to be reflected in the peak-like anomalies observed in the pressure dependences of the magnetic susceptibility at 0.26 GPa above 150 K. Our results reveal that this pressure-induced electronic state change suppresses the tetragonal-to-orthorhombic structural phase transition accompanied by an antiferromagnetic ordering. We further observed superconductivity in CaFe2As2 below ˜8 K around 0.33 GPa although our sample was not in a single phase at this pressure. These findings suggest that the electronic state change observed in CaFe2As2 with the tetragonal structure is relevant to the appearance of the pressure-induced superconductivity in AFe2As2.
NASA Astrophysics Data System (ADS)
Dubey, Sudipta; Deshmukh, Mandar M.
2016-07-01
We probe quantum Hall effect in a tunable 1-D lateral superlattice (SL) in graphene created using electrostatic gates. Lack of equilibration is observed along edge states formed by electrostatic gates inside the superlattice. We create strong local electric field at the interface of regions of different charge densities. Crossed electric and magnetic fields modify the wavefunction of the Landau Levels (LLs) - a phenomenon unique to graphene. In the region of copropagating electrons and holes at the interface, the electric field is high enough to modify the Landau levels resulting in increased scattering that tunes equilibration of edge states and this results in large longitudinal resistance.
Optical studies of 2DEGs in ZnSe quantum wells in high magnetic fields.
Ossau, Wolfgang J.; Astakhov, G. V.; Yakovlev, D. R.; Crooker, S. A.; Waag, A.
2002-01-01
Optical properties of a two-dimensional electron gas in ZnSe/(Zn,Be,Mg)Se quantum well structures have been examined by means of photoluminescence and reflectivity techniques in external magnetic fields up to 50 T. For these structures the Fermi energy of the two-dimensional electron gas is falling in the range between the trion binding energy and the exciton binding energy, which keeps the dominating role of Coulombic interaction between electrons and photoexcited holes. Characteristic peculiarities of optical spectra are discussed.
Uran, Can; Erdem, Talha; Guzelturk, Burak; Perkgöz, Nihan Kosku; Jun, Shinae; Jang, Eunjoo; Demir, Hilmi Volkan
2014-10-06
In this work, we demonstrate a proof-of-concept system for generating highly polarized light from colloidal quantum dots (QDs) coupled with magnetically aligned segmented Au/Ni/Au nanowires (NWs). Optical characterizations reveal that the optimized QD-NW coupled structures emit highly polarized light with an s-to p-polarization (s/p) contrast as high as 15:1 corresponding to a degree of polarization of 0.88. These experimental results are supported by the finite-difference time-domain simulations, which demonstrate the interplay between the inter-NW distance and the degree of polarization.
Approximate solutions to the quantum problem of two opposite charges in a constant magnetic field
NASA Astrophysics Data System (ADS)
Ardenghi, J. S.; Gadella, M.; Negro, J.
2016-05-01
We consider two particles of equal mass and opposite charge in a plane subject to a perpendicular constant magnetic field. This system is integrable but not superintegrable. From the quantum point of view, the solution is given by two fourth degree Hill differential equations which involve the energy as well as a second constant of motion. There are two solvable approximations in relation to the value of a parameter. Starting from each of these approximations, a consistent perturbation theory can be applied to get approximate values of the energy levels and of the second constant of motion.
Nonlocal magnetic configuration controlling realized in a triple-quantum-dot Josephson junction
NASA Astrophysics Data System (ADS)
Yi, Guang-Yu; Wang, Xiao-Qi; Wu, Hai-Na; Gong, Wei-Jiang
2016-07-01
We investigate the Josephson effect in a superconductor/triple-quantum-dot/superconductor junction in which the central dot is coupled to the superconductors. It is found that the supercurrent exhibits rich 0-π phase translations due to the interplay between interdot spin and electron correlations. Moreover, when the side dots are half-occupied, the nonlocal spin correlation between them, i.e., ferromagnetic or antiferromagnetic, coincides well with the supercurrent phase. We thus consider such a system to be a promising candidate for controlling the nonlocal magnetic configuration based on the Josephson effect.
Weakly relativistic quantum kinetic theory for electrostatic wave modes in magnetized plasmas
Hussain, Azhar; Stefan, Martin; Brodin, Gert
2014-03-15
We have derived the electrostatic dispersion relation in a magnetized plasma using a recently developed quantum kinetic model based on the Dirac equation. The model contains weakly relativistic spin effects such as Thomas precession, the polarization currents associated with the spin and the spin-orbit coupling. It turns out that for strictly electrostatic perturbations the non-relativistic spin effects vanish, and the modification of the classical dispersion relation is solely associated with the relativistic terms. Several new wave modes appear due the electron spin effects, and an example for astrophysical plasmas are given.
Quantum paraelectricity in copper-titanates: Magnetic-order driven vitrification
Kumar, Jitender; Awasthi, A. M.
2015-07-21
Quantum-paraelectric (QP) family character is emergent from shared low-temperature characteristics of SrCu{sub 3}Ti{sub 4}O{sub 12} (SCTO), CaCu{sub 3}Ti{sub 4}O{sub 12} (CCTO), and Ca{sub 0.9}Li{sub 0.1}Cu{sub 3}Ti{sub 4}O{sub 12} (CLCTO) A{sub 1/4}A′{sub 3/4}BO{sub 3} structures featuring antiferro-tilted Ti-O{sub 6} octahedra. Above their magnetic ordering temperatures T{sub N}, permittivity of SCTO and CLCTO follow typical Barrett form, whereas in CCTO, quantum paraelectricity is masked by the huge ε′-step. Hidden QP in CCTO gets revealed by Li-doping at the Ca-site, which considerably up-shifts the temperature scale (from ∼100 K to ∼250 K) of the dielectric step-anomaly in CLCTO. Competing magneto-electricity and quantum fluctuations result in glassy-arrest of the QP degrees of freedom near T{sub N}; manifest as dispersive-deviation of the permittivity (in SCTO and CLCTO) from the low-temperature Barrett saturation. However, quantum criticality (QC) regime being well above T{sub N} registers its presence nevertheless, as the ∼T{sup 2} behaviour of their inverse dielectric susceptibility. Non-compliance to the usual behaviours of dispersive-response vs. bias-field and temperature unambiguously rule out a relaxor origin of the glassy state. We determine a dimensionless thermal window (0.3 ≤ T/T{sub 1} ≤ 0.6) of QC signature, covering typical quantum-paraelectrics.
Kushwaha, Manvir S.
2014-12-15
Semiconducting quantum dots – more fancifully dubbed artificial atoms – are quasi-zero dimensional, tiny, man-made systems with charge carriers completely confined in all three dimensions. The scientific quest behind the synthesis of quantum dots is to create and control future electronic and optical nanostructures engineered through tailoring size, shape, and composition. The complete confinement – or the lack of any degree of freedom for the electrons (and/or holes) – in quantum dots limits the exploration of spatially localized elementary excitations such as plasmons to direct rather than reciprocal space. Here we embark on a thorough investigation of the magneto-optical absorption in semiconducting spherical quantum dots characterized by a confining harmonic potential and an applied magnetic field in the symmetric gauge. This is done within the framework of Bohm-Pines’ random-phase approximation that enables us to derive and discuss the full Dyson equation that takes proper account of the Coulomb interactions. As an application of our theoretical strategy, we compute various single-particle and many-particle phenomena such as the Fock-Darwin spectrum; Fermi energy; magneto-optical transitions; probability distribution; and the magneto-optical absorption in the quantum dots. It is observed that the role of an applied magnetic field on the absorption spectrum is comparable to that of a confining potential. Increasing (decreasing) the strength of the magnetic field or the confining potential is found to be analogous to shrinking (expanding) the size of the quantum dots: resulting into a blue (red) shift in the absorption spectrum. The Fermi energy diminishes with both increasing magnetic-field and dot-size; and exhibits saw-tooth-like oscillations at large values of field or dot-size. Unlike laterally confined quantum dots, both (upper and lower) magneto-optical transitions survive even in the extreme instances. However, the intra-Landau level
NASA Astrophysics Data System (ADS)
Kushwaha, Manvir S.
2014-12-01
Semiconducting quantum dots - more fancifully dubbed artificial atoms - are quasi-zero dimensional, tiny, man-made systems with charge carriers completely confined in all three dimensions. The scientific quest behind the synthesis of quantum dots is to create and control future electronic and optical nanostructures engineered through tailoring size, shape, and composition. The complete confinement - or the lack of any degree of freedom for the electrons (and/or holes) - in quantum dots limits the exploration of spatially localized elementary excitations such as plasmons to direct rather than reciprocal space. Here we embark on a thorough investigation of the magneto-optical absorption in semiconducting spherical quantum dots characterized by a confining harmonic potential and an applied magnetic field in the symmetric gauge. This is done within the framework of Bohm-Pines' random-phase approximation that enables us to derive and discuss the full Dyson equation that takes proper account of the Coulomb interactions. As an application of our theoretical strategy, we compute various single-particle and many-particle phenomena such as the Fock-Darwin spectrum; Fermi energy; magneto-optical transitions; probability distribution; and the magneto-optical absorption in the quantum dots. It is observed that the role of an applied magnetic field on the absorption spectrum is comparable to that of a confining potential. Increasing (decreasing) the strength of the magnetic field or the confining potential is found to be analogous to shrinking (expanding) the size of the quantum dots: resulting into a blue (red) shift in the absorption spectrum. The Fermi energy diminishes with both increasing magnetic-field and dot-size; and exhibits saw-tooth-like oscillations at large values of field or dot-size. Unlike laterally confined quantum dots, both (upper and lower) magneto-optical transitions survive even in the extreme instances. However, the intra-Landau level transitions are seen
Low-noise nano superconducting quantum interference device operating in Tesla magnetic fields.
Schwarz, Tobias; Nagel, Joachim; Wölbing, Roman; Kemmler, Matthias; Kleiner, Reinhold; Koelle, Dieter
2013-01-22
Superconductivity in the cuprate YBa(2)Cu(3)O(7) (YBCO) persists up to huge magnetic fields (B) up to several tens of Teslas, and sensitive direct current (dc) superconducting quantum interference devices (SQUIDs) can be realized in epitaxially grown YBCO films by using grain boundary Josephson junctions (GBJs). Here we present the realization of high-quality YBCO nanoSQUIDs, patterned by focused ion beam milling. We demonstrate low-noise performance of such a SQUID up to B = 1 T applied parallel to the plane of the SQUID loop at the temperature T = 4.2 K. The GBJs are shunted by a thin Au layer to provide nonhysteretic current voltage characteristics, and the SQUID incorporates a 90 nm wide constriction which is used for on-chip modulation of the magnetic flux through the SQUID loop. The white flux noise of the device increases only slightly from 1.3 μΦ(0)/(Hz)(1/2) at B = 0 to 2.3 μΦ(0)/(Hz))(1/2) at 1 T. Assuming that a point-like magnetic particle with magnetization in the plane of the SQUID loop is placed directly on top of the constriction and taking into account the geometry of the SQUID, we calculate a spin sensitivity S(μ)(1/2) = 62 μ(B)/(Hz))(1/2) at B = 0 and 110 μ(B)/(Hz))(1/2) at 1 T. The demonstration of low noise of such a SQUID in Tesla fields is a decisive step toward utilizing the full potential of ultrasensitive nanoSQUIDs for direct measurements of magnetic hysteresis curves of magnetic nanoparticles and molecular magnets. PMID:23252846
On the quantum magnetic oscillations of electrical and thermal conductivities of graphene
NASA Astrophysics Data System (ADS)
Alisultanov, Z. Z.; Reis, M. S.
2016-05-01
Oscillating thermodynamic quantities of diamagnetic materials, specially graphene, have been attracting attention of the scientific community due to the possibility to experimentally map the Fermi surface of the material. These have been the case of the de Haas-van Alphen and Shubnikov-de Haas effects, found on the magnetization and electrical conductivity, respectively. In this direction, managing the thermodynamic oscillations is of practical purpose, since from the reconstructed Fermi surface it is possible to access, for instance, the electronic density. The present work theoretically explores the quantum oscillations of electrical and thermal conductivities of a monolayer graphene under a crossed magnetic and electric fields. We found that the longitudinal electric field can increase the amplitude of the oscillations and this result is of practical and broad interest for both, experimental and device physics.
Shot noise of charge current in a quantum dot responded by rotating and oscillating magnetic fields
Zhao, Hong-Kang Zou, Wei-Ke; Chen, Qiao
2014-09-07
We have investigated the shot noise and Fano factor of the dynamic spin-polarized quantum dot under the perturbations of a rotating magnetic field (RMF), and an oscillating magnetic field (OMF) by employing the non-equilibrium Green's function approach. The shot noise is enhanced from sub-Poissonian to super-Poissonian due to the application of RMF and OMF, and it is controlled sensitively by the tilt angle θ of RMF. The magnitude of shot noise increases as the photon energy ℏω of OMF increases, and its valley eventually is reversed to peaks as the photon energy is large enough. Double-peak structure of Fano factor is exhibited as the frequency of OMF increases to cover a large regime. The Zeeman energy μ{sub 0}B{sub 0} acts as an effective gate bias to exhibit resonant behavior, and novel peak emerges associated with the applied OMF.
Eom, Byeong Ho; Penanen, Konstantin; Hahn, Inseob
2014-09-15
Magnetic resonance imaging (MRI) at microtesla fields using superconducting quantum interference device (SQUID) detection has previously been demonstrated, and advantages have been noted. Although the ultralow-field SQUID MRI technique would not need the heavy superconducting magnet of conventional MRI systems, liquid helium required to cool the low-temperature detector still places a significant burden on its operation. We have built a prototype cryocooler-based SQUID MRI system that does not require a cryogen. The SQUID detector and the superconducting gradiometer were cooled down to 3.7 K and 4.3 K, respectively. We describe the prototype design, characterization, a phantom image, and areas of further improvements needed to bring the imaging performance to parity with conventional MRI systems.
Giant effective mass deviations near the magnetic field-induced minigap in double quantum wells
Harff, N.E. |; Simmons, J.A.; Lyo, S.K.; Klem, J.F.; Goodnick, S.M.
1994-09-01
The authors report major deviations in the electron effective mass m* near the partial energy gap, or minigap, formed in strongly coupled double quantum wells (QWs) by an anticrossing of the two QW dispersion curves. The anticrossing and minigap are induced by an in-plane magnetic field B{sub {parallel}} and give rise to large distortions in the Fermi surface and density of states, including a Van Hove singularity. Sweeping B{sub {parallel}} moves the minigap through the Fermi level, with the upper and lower gap edges producing a sharp maximum and minimum in the low-temperature in-plane conductance, in agreement with theoretical calculations. The temperature dependence of Shubnikov-de Haas (SdH) oscillations appearing in a tilted magnetic field yield a decreased m* {le} 1/3 m*{sub GaAs} near the upper gap edge, and indicate an increase in m* near the lower gap edge.
Brownian motion and quantum dynamics of magnetic monopoles in spin ice
Bovo, L.; Bloxsom, J.A.; Prabhakaran, D.; Aeppli, G.; Bramwell, S.T.
2013-01-01
Spin ice illustrates many unusual magnetic properties, including zero point entropy, emergent monopoles and a quasi liquid–gas transition. To reveal the quantum spin dynamics that underpin these phenomena is an experimental challenge. Here we show how crucial information is contained in the frequency dependence of the magnetic susceptibility and in its high frequency or adiabatic limit. The typical response of Dy2Ti2O7 spin ice indicates that monopole diffusion is Brownian but is underpinned by spin tunnelling and is influenced by collective monopole interactions. The adiabatic response reveals evidence of driven monopole plasma oscillations in weak applied field, and unconventional critical behaviour in strong applied field. Our results clarify the origin of the relatively high frequency response in spin ice. They disclose unexpected physics and establish adiabatic susceptibility as a revealing characteristic of exotic spin systems. PMID:23443563
NASA Astrophysics Data System (ADS)
Pavlović, Vladan; Stevanović, Ljiljana
2016-04-01
In this paper we analyzed the realization of the electromagnetically induced transparency (EIT) effect in the spherical quantum dot with on-center hydrogenic impurity under the influence of the external magnetic field. Three energy levels of hydrogen impurity 1s0, 2p-1, and 3d-2, together with the probe and control laser fields, which induce σ- transitions between the given states, form a ladder configuration. Optical Bloch equations for such a system are solved in a stationary regime. Dependence of the susceptibility for such a system on the Rabi frequency of the control field, intensity of the external magnetic field, detuning of the control field, and decay rates coefficients are then discussed in detail. Finally, the explanation in dressed state picture is given.
Lasing and magnetic microbeads loaded with colloidal quantum dots and iron oxide nanocrystals
NASA Astrophysics Data System (ADS)
Li, Minxu; You, Guanjun; Wang, Andrew Y.; Hu, Wenjia; Wang, Jingkang; Sun, Fengqing; Zhu, Yiming; Henderson, Ron; Xu, Jian
2013-09-01
This study investigates the feasibility of loading nanostructured lasing medium and magnetic nanocrystals in the same microbead for potential applications in bio- and chemical sensing. A sequential infiltration process is proposed and tested for the preparation of magnetic and lasing microbeads by incorporating, respectively, iron oxide nanocrystals in the inner cores and colloidal quantum dots (CQDs) in the periphery regions of mesoporous silica microbeads. The co-doped bead structure was confirmed by electron microscopy and energy dispersive spectroscopy. The lasing action of the CQD gain medium in the mesoporous beads was characterized with micro-photoluminescence, revealing sharp whispering gallery mode lasing signatures, whereas the distinguishing superparamagnetic property was measured from the co-doped microbeads with vibrating sample magnetometry.
Quantum states emerging from charged transformation-wave in a uniform magnetic field
NASA Astrophysics Data System (ADS)
Lin, De-Hone
2016-06-01
It is the purpose of this paper to investigate the behavior of a charged transformation-wave in a uniform magnetic field. We first derive the equation which a transformation-wave needs to satisfy, and then, as the main application, the magnetic duality of the Hooke-Newton transmutation is performed by a conformal mapping which generates the novel states with the following characteristics: (a) bound or scattering states are classified by the signatures of the quantum number of the angular momentum and the charge of the particle; (b) the angular momentum satisfies the half-integer quantization rule; and (c) the mass parameter to reach the states is isotropic. Finally, as an alternative application, we report the construction of the fractional angular momentum and fractional Landau levels with the transformation design method.
Quantum anomalous Hall effect in atomic crystal layers from in-plane magnetization
NASA Astrophysics Data System (ADS)
Ren, Yafei; Zeng, Junjie; Deng, Xinzhou; Yang, Fei; Pan, Hui; Qiao, Zhenhua
2016-08-01
We theoretically demonstrate that with in-plane magnetization, the quantum anomalous Hall effect (QAHE) can be realized in two-dimensional atomic crystal layers with preserved inversion symmetry but broken out-of-plane mirror reflection symmetry. By taking the honeycomb lattice system as an example, we find that the low-buckled structure satisfying the symmetry criteria is crucial to induce QAHE. The topologically nontrivial bulk gap carrying a Chern number of C =±1 opens in the vicinity of the saddle points M , where the band dispersion exhibits strong anisotropy. We further show that the QAHE with electrically tunable Chern number can be achieved in Bernal-stacked multilayer systems, and the applied interlayer potential differences can dramatically decrease the critical magnetization to make the QAHE experimentally feasible.
Shot noise of charge current in a quantum dot responded by rotating and oscillating magnetic fields
NASA Astrophysics Data System (ADS)
Zhao, Hong-Kang; Zou, Wei-Ke; Chen, Qiao
2014-09-01
We have investigated the shot noise and Fano factor of the dynamic spin-polarized quantum dot under the perturbations of a rotating magnetic field (RMF), and an oscillating magnetic field (OMF) by employing the non-equilibrium Green's function approach. The shot noise is enhanced from sub-Poissonian to super-Poissonian due to the application of RMF and OMF, and it is controlled sensitively by the tilt angle θ of RMF. The magnitude of shot noise increases as the photon energy ℏω of OMF increases, and its valley eventually is reversed to peaks as the photon energy is large enough. Double-peak structure of Fano factor is exhibited as the frequency of OMF increases to cover a large regime. The Zeeman energy μ0B0 acts as an effective gate bias to exhibit resonant behavior, and novel peak emerges associated with the applied OMF.
Siderite breakdown and pressure induced Fe-C redox reactions
NASA Astrophysics Data System (ADS)
Lavina, Barbara; Dera, Przemyslaw; Kim, Eunja; Downs, Robert T.
2010-05-01
Siderite, FeCO3, was investigated at high pressure (up to ~ 40 GPa) and high temperature (up to about 2400K) using a laser heated diamond anvil cell. The structure of the sample was probed with a synchrotron monochromatic beam; powder, multigrain and single crystaldiffraction techniques were used according to changing size of the crystallites in the course of the experiment. At about 35 GPa we observed the breakdown of the carbonate into h-Fe3O4 (the orthorhombic high pressure phase of Fe3O4[1]) and undetected carbon phases. We suggest the breakdown was achieved through a redox reaction where the iron formal valence is increased at the expense of the carbon reduction. This observation is in agreement with results of shock experiments on siderite [2-4] in which however the presence of hematite in the starting material prevented to discriminate among possible reactions determining the synthesis of Fe3O4. Oxygen fugacity and the crystal chemistry of deep Earth mineral assemblages exert a major control on ionic speciation, therefore experimental confirmation are necessary to determine the actual redox equilibrium between iron and carbon in the mantle. Remarkably, perovskite strongly favor the partitioning of Fe3+ [5] and so it might favor the C reduction. If the pressure effect on Fe-C redox equilibrium found in this experiment is active in the deep Earth, the speciation of carbon would be strongly affected, in particular, the stability of carbonates and CO2 might be controlled by pressure induced reductions rather than by the stability of the pure phases. Carbon reduction at pressure might account for the greater subduction of carbon with respect to hydrogen [6]. On the other hand uplifting of reduced carbon assembly might release C-O fluids through reduction of Fe3+. Our results suggest that Fe-C redox reactions might have a crucial role on the carbon speciation which has a major importance on deep Earth processes. References [1] Haavik, et al. (2000) American
Taufour, Valentin; Kaluarachchi, Udhara S; Khasanov, Rustem; Nguyen, Manh Cuong; Guguchia, Zurab; Biswas, Pabitra Kumar; Bonfà, Pietro; De Renzi, Roberto; Lin, Xiao; Kim, Stella K; Mun, Eun Deok; Kim, Hyunsoo; Furukawa, Yuji; Wang, Cai-Zhuang; Ho, Kai-Ming; Bud'ko, Sergey L; Canfield, Paul C
2016-07-15
The temperature-pressure phase diagram of the ferromagnet LaCrGe_{3} is determined for the first time from a combination of magnetization, muon-spin-rotation, and electrical resistivity measurements. The ferromagnetic phase is suppressed near 2.1 GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFM_{Q}. Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors Q allowing for the potential of an ordering wave vector evolving from Q=0 to finite Q, as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe_{3} is a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets. PMID:27472137
Taufour, Valentin; Kaluarachchi, Udhara S.; Khasanov, Rustem; Nguyen, Manh Cuong; Guguchia, Zurab; Biswas, Pabitra Kumar; Bonfa, Pietro; De Renzi, Roberto; Lin, Xiao; Kim, Stella K.; et al
2016-07-13
Here, the temperature-pressure phase diagram of the ferromagnet LaCrGe3 is determined for the first time from a combination of magnetization, muon-spin-rotation, and electrical resistivity measurements. The ferromagnetic phase is suppressed near 2.1 GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFMQ. Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors Q allowing for the potential of an ordering wave vector evolving from Q=0 to finite Q, as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe3 ismore » a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets.« less
NASA Astrophysics Data System (ADS)
Taufour, Valentin; Kaluarachchi, Udhara S.; Khasanov, Rustem; Nguyen, Manh Cuong; Guguchia, Zurab; Biswas, Pabitra Kumar; Bonfà, Pietro; De Renzi, Roberto; Lin, Xiao; Kim, Stella K.; Mun, Eun Deok; Kim, Hyunsoo; Furukawa, Yuji; Wang, Cai-Zhuang; Ho, Kai-Ming; Bud'ko, Sergey L.; Canfield, Paul C.
2016-07-01
The temperature-pressure phase diagram of the ferromagnet LaCrGe3 is determined for the first time from a combination of magnetization, muon-spin-rotation, and electrical resistivity measurements. The ferromagnetic phase is suppressed near 2.1 GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFMQ . Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors Q allowing for the potential of an ordering wave vector evolving from Q =0 to finite Q , as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe3 is a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets.
Squeezed-state source using radiation-pressure-induced rigidity
Corbitt, Thomas; Ottaway, David; Mavalvala, Nergis; Chen Yanbei; Khalili, Farid; Vyatchanin, Sergey; Whitcomb, Stan
2006-02-15
We propose an experiment to extract ponderomotive squeezing from an interferometer with high circulating power and low mass mirrors. In this interferometer, optical resonances of the arm cavities are detuned from the laser frequency, creating a mechanical rigidity that dramatically suppresses displacement noises. After taking into account imperfection of optical elements, laser noise, and other technical noise consistent with existing laser and optical technologies and typical laboratory environments, we expect the output light from the interferometer to have measurable squeezing of 5 dB, with a frequency-independent squeeze angle for frequencies below 1 kHz. This squeeze source is well suited for injection into a gravitational-wave interferometer, leading to improved sensitivity from reduction in the quantum noise. Furthermore, this design provides an experimental test of quantum-limited radiation pressure effects, which have not previously been tested.
Pressure induced metallization of the perovskite Sr{sub 3}Fe{sub 2}O{sub 7}
Rozenberg, G.K.; Machavariani, G.Y.; Pasternak, M.P.; Milner, A.P.; Hearne, G.R.; Taylor, R.D.; Adler, P.
1998-12-31
Electrical, magnetic and structural properties of the antiferromagnetic semiconductor Sr{sub 3}Fe{sub 2}O{sub 7} (Fe{sup 4+}, d{sup 4}) were probed by resistance, Moessbauer spectroscopy (MS) and X-ray diffraction (XRD) measurements to P {approximately} 40 GPa using diamond-anvil cells. A sluggish pressure-induced insulator-metal transition is observed with a clear incipient metallic state at P {ge} 20 GPa. The Fe(IV) 3d magnetic moments remain unaltered across the transition as deduced from MS, and XRD studies show no structural symmetry change to 40 GPa. The results are consistent with carrier delocalization due to p-p gap closure e.g., ligand-to-ligand charge transfer that does not involve the d-states and structural symmetry changes.
Wu, Wei
2014-07-23
The magnetic properties of a theoretically designed molecular chain structure CuCoPc2, in which copper-phthalocyanine (CuPc) and cobalt-phthalocyanine (CoPc) alternate, have been investigated across a range of chain structures. The computed exchange interaction for the α-phase CuCoPc2 is ∼ 5 K (ferromagnetic), in strong contrast to the anti-ferromagnetic interaction recently observed in CuPc and CoPc. The computed exchange interactions are strongly dependent on the stacking angle but weakly on the sliding angle, and peak at 20 K (ferromagnetic). These ferromagnetic interactions are expected to arise from direct exchange with the strong suppression of super-exchange interaction. These first-principles calculations show that π-conjugated molecules, such as phthalocyanine, could be used as building blocks for the design of magnetic materials. This therefore extends the concept of quantum metamaterials further into magnetism. The resulting new magnetic materials could find applications in the studies such as organic spintronics. PMID:24990182
Magnetic control of Rashba splittings in symmetric InAs quantum wells
NASA Astrophysics Data System (ADS)
Matsuura, Toru; Faniel, Sébastien; Monta, Nozomu; Koga, Takaaki
2010-09-01
We propose a mechanism to control the Rashba-induced subband splitting by a magnetic field using a symmetric double quantum well (QW) system, where the lowest two subbands are coupled by a position-dependent Rashba parameter α(z). In such a system, all subbands are spin degenerate due to the time reversal symmetry and the spatial inversion symmetry at zero magnetic field, despite the presence of the Rashba spin-orbit interaction. Applying an external magnetic field parallel to the QW plane ( B∥y^) lifts this spin degeneracy breaking the time reversal symmetry, where the spin splitting energies are controllable in the range between zero and 2.9 meV, the latter being on the same order of magnitude as a typical Rashba splitting in a narrow asymmetric QW. We find that the first and second subband energy levels for a selected spin state with k∥=(kF,0,0) anticross each other, and that the energy of the subband splitting Δ0, equivalent to the Rashba splitting for the case of single QWs, can be determined from the value of the anticrossing magnetic field Bac. These results suggest that the investigation in the symmetric double QWs would provide useful approaches for quantitative understanding of the Rashba spin-orbit interaction.
Optical signatures of electric-field-driven magnetic phase transitions in graphene quantum dots
NASA Astrophysics Data System (ADS)
Basak, Tista; Shukla, Alok
2016-06-01
Experimental challenges in identifying various types of magnetic ordering in graphene quantum dots (QDs) pose a major hurdle in the application of these nanostructures for spintronic devices. Based upon phase diagrams obtained by employing the π -electron Pariser-Parr-Pople (PPP) model Hamiltonian, we demonstrate that the magnetic states undergo phase transition under the influence of an external electric field. Our calculations of the electroabsorption spectra of these QDs indicate that the spectrum in question carries strong signatures of their magnetic state (FM vs AFM), thus suggesting the possibility of an all-optical characterization of their magnetic nature. Further, the gaps for the up and the down spins are the same in the absence of an external electric field, both for the antiferromagnetic (AFM) and the ferromagnetic (FM) states of QDs. But, once the QDs are exposed to a suitably directed external electric field, gaps for different spins split and exhibit distinct variations with respect to the strength of the field. The nature of variation exhibited by the energy gaps corresponding to the up and down spins is different for the AFM and FM configurations of QDs. This selective manipulation of the spin-polarized gap splitting by an electric field in finite graphene nanostructures can open up new frontiers in the design of graphene-based spintronic devices.
Experimental exploration over a quantum control landscape through nuclear magnetic resonance
NASA Astrophysics Data System (ADS)
Sun, Qiuyang; Pelczer, István; Riviello, Gregory; Wu, Re-Bing; Rabitz, Herschel
2014-03-01
The growing successes in performing quantum control experiments motivated the development of control landscape analysis as a basis to explain these findings. When a quantum system is controlled by an electromagnetic field, the observable as a functional of the control field forms a landscape. Theoretical analyses have revealed many properties of control landscapes, especially regarding their slopes, curvatures, and topologies. A full experimental assessment of the landscape predictions is important for future consideration of controlling quantum phenomena. Nuclear magnetic resonance (NMR) is exploited here as an ideal laboratory setting for quantitative testing of the landscape principles. The experiments are performed on a simple two-level proton system in a H2O-D2O sample. We report a variety of NMR experiments roving over the control landscape based on estimation of the gradient and Hessian, including ascent or descent of the landscape, level set exploration, and an assessment of the theoretical predictions on the structure of the Hessian. The experimental results are fully consistent with the theoretical predictions. The procedures employed in this study provide the basis for future multispin control landscape exploration where additional features are predicted to exist.
Quantum spin ices and magnetic states from dipolar-octupolar doublets on the pyrochlore lattice
NASA Astrophysics Data System (ADS)
Chen, Gang
We consider a class of electron systems in which dipolar-octupolar Kramers doublets arise on the pyrochlore lattice. In the localized limit, the Kramers doublets are described by the effective spin 1/2 pseudospins. The most general nearest-neighbor exchange model between these pseudospins is the XYZ model. In additional to dipolar ordered and octupolar ordered magnetic states, we show that this XYZ model exhibits two distinct quantum spin ice (QSI) phases, that we dub dipolar QSI and octupolar QSI. These two QSIs are distinct symmetry enriched U(1) quantum spin liquids, enriched by the lattice symmetry. Moreover, the XYZ model is absent from the notorious sign problem for a quantum Monte Carlo simulation in a large parameter space. We discuss the potential relevance to real material systems such as Dy2Ti2O7, Nd2Zr2O7, Nd2Hf2O7, Nd2Ir2O7, Nd2Sn2O7 and Ce2Sn2O7. chggst@gmail.com, Refs: Y-P Huang, G Chen, M Hermele, Phys. Rev. Lett. 112, 167203 (2014).
Manipulation of the nuclear spin ensemble in a quantum dot with chirped magnetic resonance pulses
NASA Astrophysics Data System (ADS)
Munsch, Mathieu; Wüst, Gunter; Kuhlmann, Andreas V.; Xue, Fei; Ludwig, Arne; Reuter, Dirk; Wieck, Andreas D.; Poggio, Martino; Warburton, Richard J.
2014-09-01
The nuclear spins in nanostructured semiconductors play a central role in quantum applications. The nuclear spins represent a useful resource for generating local magnetic fields but nuclear spin noise represents a major source of dephasing for spin qubits. Controlling the nuclear spins enhances the resource while suppressing the noise. NMR techniques are challenging: the group III and V isotopes have large spins with widely different gyromagnetic ratios; in strained material there are large atom-dependent quadrupole shifts; and nanoscale NMR is hard to detect. We report NMR on 100,000 nuclear spins of a quantum dot using chirped radiofrequency pulses. Following polarization, we demonstrate a reversal of the nuclear spin. We can flip the nuclear spin back and forth a hundred times. We demonstrate that chirped NMR is a powerful way of determining the chemical composition, the initial nuclear spin temperatures and quadrupole frequency distributions for all the main isotopes. The key observation is a plateau in the NMR signal as a function of sweep rate: we achieve inversion at the first quantum transition for all isotopes simultaneously. These experiments represent a generic technique for manipulating nanoscale inhomogeneous nuclear spin ensembles and open the way to probe the coherence of such mesoscopic systems.
Pressure induced structural phase transition in IB transition metal nitrides compounds
NASA Astrophysics Data System (ADS)
Soni, Shubhangi; Kaurav, Netram; Jain, A.; Shah, S.; Choudhary, K. K.
2015-06-01
Transition metal mononitrides are known as refractory compounds, and they have, relatively, high hardness, brittleness, melting point, and superconducting transition temperature, and they also have interesting optical, electronic, catalytic, and magnetic properties. Evolution of structural properties would be an important step towards realizing the potential technological scenario of this material of class. In the present study, an effective interionic interaction potential (EIOP) is developed to investigate the pressure induced phase transitions in IB transition metal nitrides TMN [TM = Cu, Ag, and Au] compounds. The long range Coulomb, van der Waals (vdW) interaction and the short-range repulsive interaction upto second-neighbor ions within the Hafemeister and Flygare approach with modified ionic charge are properly incorporated in the EIOP. The vdW coefficients are computed following the Slater-Kirkwood variational method, as both the ions are polarizable. The estimated value of the phase transition pressure (Pt) and the magnitude of the discontinuity in volume at the transition pressure are consistent as compared to the reported data.
Pressure induced structural phase transition in IB transition metal nitrides compounds
Soni, Shubhangi; Kaurav, Netram Jain, A.; Shah, S.; Choudhary, K. K.
2015-06-24
Transition metal mononitrides are known as refractory compounds, and they have, relatively, high hardness, brittleness, melting point, and superconducting transition temperature, and they also have interesting optical, electronic, catalytic, and magnetic properties. Evolution of structural properties would be an important step towards realizing the potential technological scenario of this material of class. In the present study, an effective interionic interaction potential (EIOP) is developed to investigate the pressure induced phase transitions in IB transition metal nitrides TMN [TM = Cu, Ag, and Au] compounds. The long range Coulomb, van der Waals (vdW) interaction and the short-range repulsive interaction upto second-neighbor ions within the Hafemeister and Flygare approach with modified ionic charge are properly incorporated in the EIOP. The vdW coefficients are computed following the Slater-Kirkwood variational method, as both the ions are polarizable. The estimated value of the phase transition pressure (Pt) and the magnitude of the discontinuity in volume at the transition pressure are consistent as compared to the reported data.
Bonev, B B; Morrow, M R
1995-01-01
The effects of pressure and temperature on 1,2-dipalmitoyl-sn-glycero-3-phosphocholine and 1,2-dimyristoyl-sn-glycero-3-phosphocholine headgroup conformations were examined using deuterium nuclear magnetic resonance. Isothermal compression was found to produce a decrease in the choline alpha deuteron quadrupole splitting and increases in the choline beta and gamma deuteron quadrupole splittings. A similar counterdirectional change, seen in the presence of positive surface charge, has been attributed to tilting of the headgroup away from the bilayer surface in response to the torque exerted on the phosphocholine dipole by positive surface charges. The direction of the change in headgroup deuteron quadrupole splitting is consistent with the pressure-induced reduction in area per lipid in the liquid crystalline phase, which can be inferred from the ordering of phospholipid acyl chains under comparable conditions. The temperature dependences of the headgroup deuteron quadrupole splittings were also examined. It was found that at elevated pressure, the alpha splitting was insensitive to temperature, whereas the beta and gamma splittings decreased. The response of the beta deuteron splitting to temperature was found to be weaker at elevated pressure than at ambient pressure. PMID:8527666
Bonev, B B; Morrow, M R
1995-08-01
The effects of pressure and temperature on 1,2-dipalmitoyl-sn-glycero-3-phosphocholine and 1,2-dimyristoyl-sn-glycero-3-phosphocholine headgroup conformations were examined using deuterium nuclear magnetic resonance. Isothermal compression was found to produce a decrease in the choline alpha deuteron quadrupole splitting and increases in the choline beta and gamma deuteron quadrupole splittings. A similar counterdirectional change, seen in the presence of positive surface charge, has been attributed to tilting of the headgroup away from the bilayer surface in response to the torque exerted on the phosphocholine dipole by positive surface charges. The direction of the change in headgroup deuteron quadrupole splitting is consistent with the pressure-induced reduction in area per lipid in the liquid crystalline phase, which can be inferred from the ordering of phospholipid acyl chains under comparable conditions. The temperature dependences of the headgroup deuteron quadrupole splittings were also examined. It was found that at elevated pressure, the alpha splitting was insensitive to temperature, whereas the beta and gamma splittings decreased. The response of the beta deuteron splitting to temperature was found to be weaker at elevated pressure than at ambient pressure. PMID:8527666
Vezzalini, Giovanna; Arletti, Rossella; Quartieri, Simona
2014-06-01
This is a comparative study on the high-pressure behavior of microporous materials with an MFI framework type (i.e. natural mutinaite, ZSM-5 and the all-silica phase silicalite-1), based on in-situ experiments in which penetrating and non-penetrating pressure-transmitting media were used. Different pressure-induced phenomena and deformation mechanisms (e.g. pressure-induced over-hydration, pressure-induced amorphization) are discussed. The influence of framework and extra-framework composition and of the presence of silanol defects on the response to the high pressure of MFI-type zeolites is discussed. PMID:24892591
NASA Astrophysics Data System (ADS)
Lai, Wenxi; Yang, Wen
2015-10-01
We consider theoretically a magnetic impurity spin driven by polarized electrons tunneling through a double-quantum-dot system. The spin-blockade effect and spin conservation in the system make the magnetic impurity sufficiently interact with each transferring electron. As a result, a single collected electron carries information about spin change of the magnetic impurity. The scheme may develop all-electrical manipulation of magnetic atoms by means of single electrons, which is significant for the implementation of scalable logical gates in information processing systems.
Continuous and discontinuous quantum phase transitions in a model two-dimensional magnet
Haravifard, S.; Banerjee, A.; Lang, J. C.; Srajer, G.; Silevitch, D. M.; Gaulin, B. D.; Dabkowska, H. A.; Rosenbaum, T. F.
2012-01-01
The Shasty–Sutherland model, which consists of a set of spin 1/2 dimers on a 2D square lattice, is simple and soluble but captures a central theme of condensed matter physics by sitting precariously on the quantum edge between isolated, gapped excitations and collective, ordered ground states. We compress the model Shastry–Sutherland material, SrCu2(BO3)2, in a diamond anvil cell at cryogenic temperatures to continuously tune the coupling energies and induce changes in state. High-resolution X-ray measurements exploit what emerges as a remarkably strong spin-lattice coupling to both monitor the magnetic behavior and the absence or presence of structural discontinuities. In the low-pressure spin-singlet regime, the onset of magnetism results in an expansion of the lattice with decreasing temperature, which permits a determination of the pressure-dependent energy gap and the almost isotropic spin-lattice coupling energies. The singlet-triplet gap energy is suppressed continuously with increasing pressure, vanishing completely by 2 GPa. This continuous quantum phase transition is followed by a structural distortion at higher pressure. PMID:22308373
Continuous and discontinuous quantum phase transitions in a model two-dimensional magnet.
Haravifard, S; Banerjee, A; Lang, J C; Srajer, G; Silevitch, D M; Gaulin, B D; Dabkowska, H A; Rosenbaum, T F
2012-02-14
The Shasty-Sutherland model, which consists of a set of spin 1/2 dimers on a 2D square lattice, is simple and soluble but captures a central theme of condensed matter physics by sitting precariously on the quantum edge between isolated, gapped excitations and collective, ordered ground states. We compress the model Shastry-Sutherland material, SrCu(2)(BO(3))(2), in a diamond anvil cell at cryogenic temperatures to continuously tune the coupling energies and induce changes in state. High-resolution X-ray measurements exploit what emerges as a remarkably strong spin-lattice coupling to both monitor the magnetic behavior and the absence or presence of structural discontinuities. In the low-pressure spin-singlet regime, the onset of magnetism results in an expansion of the lattice with decreasing temperature, which permits a determination of the pressure-dependent energy gap and the almost isotropic spin-lattice coupling energies. The singlet-triplet gap energy is suppressed continuously with increasing pressure, vanishing completely by 2 GPa. This continuous quantum phase transition is followed by a structural distortion at higher pressure. PMID:22308373
NASA Astrophysics Data System (ADS)
Ostahie, B.; Aldea, A.
2016-02-01
Spectral and transport properties of electrons in confined phosphorene systems are investigated in a five hopping parameter tight-binding model, using analytical and numerical techniques. The main emphasis is on the properties of the topological edge states accommodated by the quasiflat band that characterizes the phosphorene energy spectrum. We show, in the particular case of phosphorene, how the breaking of the bipartite lattice structure gives rise to the electron-hole asymmetry of the energy spectrum. The properties of the topological edge states in the zigzag nanoribbons are analyzed under different aspects: degeneracy, localization, extension in the Brillouin zone, dispersion of the quasiflat band in magnetic field. The finite-size phosphorene plaquette exhibits a Hofstadter-type spectrum made up of two unequal butterflies separated by a gap, where a quasiflat band composed of zigzag edge states is located. The transport properties are investigated by simulating a four-lead Hall device (importantly, all leads are attached on the same zigzag side), and using the Landauer-Büttiker formalism. We find out that the chiral edge states due to the magnetic field yield quantum Hall plateaus, but the topological edge states in the gap do not support the quantum Hall effect and prove a dissipative behavior. By calculating the complex eigenenergies of the non-Hermitian effective Hamiltonian that describes the open system (plaquette+leads), we prove the superradiance effect in the energy range of the quasiflat band, with consequences for the density of states and electron transmission properties.
Intrinsic Localized Modes in Quantum Ferromagnetic XXZ Chains in an Oblique Magnetic Field
NASA Astrophysics Data System (ADS)
Li, De-Jun
2016-02-01
A semiclassical study of intrinsic localized spin-wave modes in a one-dimensional quantum ferromagnetic XXZ chain in an oblique magnetic field is presented in this paper. We quantize the model Hamiltonian by introducing the Dyson-Maleev transformation, and adopt the coherent state representation as the basic representation of the system. By means of the method of multiple scales combined with a quasidiscreteness approximation, the equation of motion for the coherent-state amplitude can be reduced to the standard nonlinear Schrödinger equation. It is found that, at the center of the Brillouin zone, when θ < θ c a bright intrinsic localized spin-wave mode appears below the bottom of the magnon frequency band and when θ > θ c a dark intrinsic localized spin-wave resonance mode can occur above the bottom of the magnon frequency band. In other words, the switch between the bright and dark intrinsic localized spin-wave modes can be controlled via varying the angle of the magnetic field. This result has potential applications in quantum information storage. In addition, we find that, at the boundary of the Brillouin zone, the system can only produce a dark intrinsic localized spin-wave mode, whose eigenfrequency is above the upper of the magnon frequency band.
Exchange interactions in CdMnTe/CdMgTe quantum wells under high magnetic fields
NASA Astrophysics Data System (ADS)
Yasuhira, T.; Uchida, K.; Matsuda, Y. H.; Miura, N.; Kuroda, S.; Takita, K.
2002-03-01
The sp-d exchange interaction Jsp-d and the exchange interaction between the nearest neighbor Mn ions JNN were studied by magneto-photoluminescence spectra of excitons in CdMnTe/CdMgTe quantum wells in pulsed high magnetic fields up to 45 T. The magnitude of Jsp-d estimated from the observed Zeeman splitting was found to decrease as the quantum well width was decreased. The decrease is partly due to the penetration of the electron and the hole wave functions into the non-magnetic CdMgTe barrier layers, and partly due to the k-dependence of the exchange interaction. It was found that the latter effect is much larger than theoretically predicted. The observed features are well explained by a model assuming the interface disorder within some thickness near the interface. In contrast to Jsp-d, the nearest neighbor interaction JNN estimated from the steps in the photoluminescence peak was found to be independent of the well width.
Local dissipation effects in two-dimensional quantum Josephson junction arrays with a magnetic field
Polak, T.P.; Kopec, T.K.
2005-07-01
We study the quantum phase transitions in two-dimensional arrays of Josephson-couples junctions with short range Josephson couplings (given by the Josephson energy E{sub J}) and the charging energy E{sub C}. We map the problem onto the solvable quantum generalization of the spherical model that improves over the mean-field theory method. The arrays are placed on the top of a two-dimensional electron gas separated by an insulator. We include effects of the local dissipation in the presence of an external magnetic flux f={phi}/{phi}{sub 0} in square lattice for several rational fluxes f=0,(1/2),(1/3),(1/4), and (1/6). We also have examined the T=0 superconducting-insulator phase boundary as a function of a dissipation {alpha}{sub 0} for two different geometry of the lattice: square and triangular. We have found a critical value of the dissipation parameter independent on geometry of the lattice and presence magnetic field.
Anomalous Dynamical Line Shapes in a Quantum Magnet at Finite Temperature
Tennant D. A.; James A.; Lake, B.; Essler, F.H.L.; Notbohm, S.; Mikeska, H.-J.; Fielden, J.; Kogerler,, P.; Canfield, P.C.; Telling, M.T.F.
2012-01-04
The effect of thermal fluctuations on the dynamics of a gapped quantum magnet is studied using inelastic neutron scattering on copper nitrate, a model material for the spin-1/2, one-dimensional (1D) bond alternating Heisenberg chain. A large, highly deuterated, single-crystal sample of copper nitrate is produced using a solution growth method and measurements are made using the high-resolution backscattering spectrometer OSIRIS at the ISIS Facility. Theoretical calculations and numerical analysis are combined to interpret the physical origin of the thermal effects observed in the magnetic spectra. The primary observations are (1) a thermally induced central peak due to intraband scattering, which is similar to Villain scattering familiar from soliton systems in 1D, and (2) the one-magnon quasiparticle pole is seen to develop with temperature into an asymmetric continuum of scattering. We relate this asymmetric line broadening to a thermal strongly correlated state caused by hard-core constraints and quasiparticle interactions. These findings are a counter example to recent assertions of the universality of line broadening in 1D systems and are applicable to a broad range of quantum systems.
Anomalous dynamical line shapes in a quantum magnet at finite temperature
NASA Astrophysics Data System (ADS)
Tennant, D. A.; Lake, B.; James, A. J. A.; Essler, F. H. L.; Notbohm, S.; Mikeska, H.-J.; Fielden, J.; Kögerler, P.; Canfield, P. C.; Telling, M. T. F.
2012-01-01
The effect of thermal fluctuations on the dynamics of a gapped quantum magnet is studied using inelastic neutron scattering on copper nitrate, a model material for the spin-1/2, one-dimensional (1D) bond alternating Heisenberg chain. A large, highly deuterated, single-crystal sample of copper nitrate is produced using a solution growth method and measurements are made using the high-resolution backscattering spectrometer OSIRIS at the ISIS Facility. Theoretical calculations and numerical analysis are combined to interpret the physical origin of the thermal effects observed in the magnetic spectra. The primary observations are (1) a thermally induced central peak due to intraband scattering, which is similar to Villain scattering familiar from soliton systems in 1D, and (2) the one-magnon quasiparticle pole is seen to develop with temperature into an asymmetric continuum of scattering. We relate this asymmetric line broadening to a thermal strongly correlated state caused by hard-core constraints and quasiparticle interactions. These findings are a counter example to recent assertions of the universality of line broadening in 1D systems and are applicable to a broad range of quantum systems.
Carrier relaxation in (In,Ga)As quantum dots with magnetic field-induced anharmonic level structure
NASA Astrophysics Data System (ADS)
Kurtze, H.; Bayer, M.
2016-07-01
Sophisticated models have been worked out to explain the fast relaxation of carriers into quantum dot ground states after non-resonant excitation, overcoming the originally proposed phonon bottleneck. We apply a magnetic field along the quantum dot heterostructure growth direction to transform the confined level structure, which can be approximated by a Fock-Darwin spectrum, from a nearly equidistant level spacing at zero field to strong anharmonicity in finite fields. This changeover leaves the ground state carrier population rise time unchanged suggesting that fast relaxation is maintained upon considerable changes of the level spacing. This corroborates recent models explaining the relaxation by polaron formation in combination with quantum kinetic effects.
Inter-layer frictional drag in double quantum wells in perpendicular magnetic fields
NASA Astrophysics Data System (ADS)
Feng, Xiang Guang
Friction drag between isolated two-dimensional electron gas (2DEG) layers is a relatively new experimental probe for the study of the inter-layer interactions of two-dimensional electron systems. By measuring drag as a function of various experimental parameters we can explore details of the electron-electron interactions and gain insight into the electronic states. As many new and interesting phenomena have been discovered for two-dimensional electron gas systems in magnetic fields, beginning with the discovery of the quantum Hall-effect, we were motivated to measure drag in magnetic fields perpendicular to the 2DEG. In our drag experiment in magnetic fields, we observed two unusual phenomena. First in intermediate field range, where the Landau level splitting is smaller than the thermal energy kT, we observed an unusual increase in drag in intermediate fields, which cannot be explained by current theory based on single particle scattering. We think the cause of this unusual increase is related to inter-layer correlation induced by magnetic field. Secondly, in strong magnetic fields and unmatched layer densities, we observed negative drag peaks at certain field values, which have opposite polarity to the drag of electron-electron system at zero field. We argue that the negative drag reveals unusual dispersion of the electronic states near the Landau level, in which electrons show hole-like behavior. We hope our work can inspire more studies, both theoretically and experimentally, on the two dimensional electron systems in magnetic field. The experiments discussed here were performed in Dr. Gramila's research group in the department of physics of Pennsylvania State University.
NASA Astrophysics Data System (ADS)
Ge, Song
In this dissertation, I present the development of a SQUID (Superconducting Quantum Interference Device) imaging system using targeted magnetic nanoparticles (NPs) as contrast agents. The contrast agents are functionalized for targeting by the conjugation of the magnetic NPs to folic acid (FA) molecules on dendrimer scaffolds. Cellular internalization is accomplished through the high-affinity folic acid receptors (FARs), which are overexpressed in various human carcinomas. SQUID can be applied to detect signals from the magnetic cores of the contrast agents and hence diagnose the tumor. Based on the magnetic properties of the magnetic NPs, two detection methods were developed: remanence and magnetorelaxometry (MRX). The remanence measurement-based method detects magnetic NPs that are sufficiently large and possess long relaxation time. Samples were vertically oscillated and horizontally translated each in one-dimension. The system was calibrated with gamma-Fe2O3 NPs (mean diameter 25 nm) and the detection limit was found to be 10 ng at a distance of 1.7 cm and the spatial resolution was ˜1 cm. A theoretical model of this system was proposed and applied to image reconstruction of scanned phantoms with two NP injection spots. The developed SQUID system can determine not only the amount and horizontal position of the NPs, but also their depth in the phantoms. The MRX technique utilizes the NPs superparamagnetic property and records their time course magnetic decay. The system was investigated by using a number of iron oxide NP products with different mean diameters. The results showed that the MRX signal intensity is sensitively dependent on the size of the NPs. The best detection limit of 300 ng of total iron content was found on using a d = 12 nm Fe3O4 NP sample and this result was supported by computer simulations. To produce magnetic NPs for the MRX study, a synthetic approach of size-controllable Fe3O4 NPs was developed. Accordingly, the magnetic property can be
Ding, Ke; Jing, Lihong; Liu, Chunyan; Hou, Yi; Gao, Mingyuan
2014-02-01
Magnetically engineered Cd-free CuInS2@ZnS:Mn quantum dots (QDs) were designed, synthesized, and evaluated as potential dual-modality probes for fluorescence and magnetic resonance imaging (MRI) of tumors in vivo. The synthesis of Mn-doped core-shell structured CuInS2@ZnS mainly comprised three steps, i.e., the preparation of fluorescent CuInS2 seeds, the particle surface coating of ZnS, and the Mn-doping of the ZnS shells. Systematic spectroscopy studies were carried out to illustrate the impacts of ZnS coating and the following Mn-doping on the optical properties of the QDs. In combination with conventional fluorescence, fluorescence excitation, and time-resolved fluorescence measurements, the structure of CuInS2@ZnS:Mn QDs prepared under optimized conditions presented a Zn gradient CuInS2 core and a ZnS outer shell, while Mn ions were mainly located in the ZnS shell, which well balanced the optical and magnetic properties of the resultant QDs. For the following in vivo imaging experiments, the hydrophobic CuInS2@ZnS:Mn QDs were transferred into water upon ligand exchange reactions by replacing the 1-dodecanethiol ligand with dihydrolipoic acid-poly(ethylene glycol) (DHLA-PEG) ligand. The MTT assays based on HeLa cells were carried out to evaluate the cytotoxicity of the current Cd-free CuInS2@ZnS:Mn QDs for comparing with that of water soluble CdTe QDs. Further in vivo fluorescence and MR imaging experiments suggested that the PEGylated CuInS2@ZnS:Mn QDs could well target both subcutaneous and intraperitoneal tumors in vivo. PMID:24239108
Tokiwa, Y.; Yamashita, T.; Udagawa, M.; Kittaka, S.; Sakakibara, T; Terazawa, D.; Shimoyama, Y.; Terashima, T.; Yasui, Y.; Shibauchi, T.; Matsuda, Y.
2016-01-01
The low-energy elementary excitations in frustrated quantum magnets have fascinated researchers for decades. In frustrated Ising magnets on a pyrochlore lattice possessing macroscopically degenerate spin-ice ground states, the excitations have been discussed in terms of classical magnetic monopoles, which do not contain quantum fluctuations. Here we report unusual behaviours of magneto-thermal conductivity in the disordered spin-liquid regime of pyrochlore Yb2Ti2O7, which hosts frustrated spin-ice correlations with large quantum fluctuations owing to pseudospin-1/2 of Yb ions. The analysis of the temperature and magnetic field dependencies shows the presence of gapped elementary excitations. We find that the gap energy is largely suppressed from that expected in classical monopoles. Moreover, these excitations propagate a long distance without being scattered, in contrast to the diffusive nature of classical monopoles. These results suggests the emergence of highly itinerant quantum magnetic monopole, which is a heavy quasiparticle that propagates coherently in three-dimensional spin liquids. PMID:26912080
Masuda, Hidetoshi; Sakai, Hideaki; Tokunaga, Masashi; Yamasaki, Yuichi; Miyake, Atsushi; Shiogai, Junichi; Nakamura, Shintaro; Awaji, Satoshi; Tsukazaki, Atsushi; Nakao, Hironori; Murakami, Youichi; Arima, Taka-hisa; Tokura, Yoshinori; Ishiwata, Shintaro
2016-01-01
For the innovation of spintronic technologies, Dirac materials, in which low-energy excitation is described as relativistic Dirac fermions, are one of the most promising systems because of the fascinating magnetotransport associated with extremely high mobility. To incorporate Dirac fermions into spintronic applications, their quantum transport phenomena are desired to be manipulated to a large extent by magnetic order in a solid. We report a bulk half-integer quantum Hall effect in a layered antiferromagnet EuMnBi2, in which field-controllable Eu magnetic order significantly suppresses the interlayer coupling between the Bi layers with Dirac fermions. In addition to the high mobility of more than 10,000 cm(2)/V s, Landau level splittings presumably due to the lifting of spin and valley degeneracy are noticeable even in a bulk magnet. These results will pave a route to the engineering of magnetically functionalized Dirac materials. PMID:27152326
Masuda, Hidetoshi; Sakai, Hideaki; Tokunaga, Masashi; Yamasaki, Yuichi; Miyake, Atsushi; Shiogai, Junichi; Nakamura, Shintaro; Awaji, Satoshi; Tsukazaki, Atsushi; Nakao, Hironori; Murakami, Youichi; Arima, Taka-hisa; Tokura, Yoshinori; Ishiwata, Shintaro
2016-01-01
For the innovation of spintronic technologies, Dirac materials, in which low-energy excitation is described as relativistic Dirac fermions, are one of the most promising systems because of the fascinating magnetotransport associated with extremely high mobility. To incorporate Dirac fermions into spintronic applications, their quantum transport phenomena are desired to be manipulated to a large extent by magnetic order in a solid. We report a bulk half-integer quantum Hall effect in a layered antiferromagnet EuMnBi2, in which field-controllable Eu magnetic order significantly suppresses the interlayer coupling between the Bi layers with Dirac fermions. In addition to the high mobility of more than 10,000 cm2/V s, Landau level splittings presumably due to the lifting of spin and valley degeneracy are noticeable even in a bulk magnet. These results will pave a route to the engineering of magnetically functionalized Dirac materials. PMID:27152326
NASA Astrophysics Data System (ADS)
Kamiya, Yoshitomo
The possibility of quantum spin liquids, characterized by nontrivial entanglement properties or a topological nonlocal order parameter, has long been debated both theoretically and experimentally. Since candidate systems (e.g., frustrated quantum magnets or 5 d transition metal oxides) may host other competing phases including conventional magnetic ordered phases, it is natural to ask what types of global phase diagrams can be anticipated depending on coupling constants, temperature, dimensionality, etc. In this talk, by considering an extension of the Kitaev toric code Hamiltonians by Ising interactions on 2D (square) and 3D (cubic) lattices, I will present thermodynamic phase diagrams featuring magnetic ``three states of matter,'' namely, quantum spin liquid, paramagnetic, and magnetically ordered phases (analogous to liquid, gas, and solid, respectively, in conventional matter) obtained by unbiased quantum Monte Carlo simulations [YK, Y. Kato, J. Nasu, and Y. Motome, PRB 92, 100403(R) (2015)]. We find that the ordered phase borders on the spin liquid around the exactly solvable point by a discontinuous transition line in 3D, while it grows continuously from the quantum critical point in 2D. In both cases, peculiar proximity effects to the nearby spin liquid phases are observed at high temperature even when the ground state is magnetically ordered. Such proximity effects include flux-shrinking and a tricritical behavior in 3D and a ``fractionalization'' of the order parameter field at the quantum critical point in 2D, both of which can be detected by measuring critical exponents. Work done in collaboration with Yasuyuki Kato, Joji Nasu, and Yukitoshi Motome.
Pressure-driven high to low spin transition in the bimetallic quantum magnet [Ru2(O2CMe)4]3[Cr(CN)6
O'Neal, K. R.; Liu, Z.; Miller, Joel S.; Fishman, Randy Scott; Musfeldt, J. L.
2014-01-01
Synchrotron-based infrared and Raman spectroscopies were brought together with diamond anvil cell techniques and an analysis of the magnetic properties to investigate the pressure-induced high low spin transition in [Ru2(O2CMe)4]3[Cr(CN)6]. The extended nature of the diruthenium wavefunction combined with coupling to chromium-related local lattice distortions changes the relative energies of the and orbitals and drives the high low spin transition on the mixed-valence diruthenium complex. This is a rare example of an externally controlled metamagnetic transition in which both spin-orbit and spin-lattice interactions contribute to the mechanism.
Modeling of magnetic polaron properties in (Zn,Mn)Te quantum dots
NASA Astrophysics Data System (ADS)
Pientka, James; Barman, B.; Schweidenback, L.; Russ, A. H.; Tsai, Y.; Murphy, J. R.; Cartwright, A. N.; Zutic, I.; McCombe, B. D.; Petrou, A.; Chou, W.-C.; Fan, W. C.; Sellers, I. R.; Petukhov, A. G.; Oszwaldowski, R.
Magnetic polarons in (Zn,Mn)Te quantum dots (QD) show unconventional behavior. These structures exhibit a small red shift of the photoluminescence peak energy in the presence of a magnetic field B and they also have a weak dependence of the polaron energy EMP on temperature T and B. We attribute these properties to a large molecular field Bm that is proportional to the heavy holes spin density. We have calculated Bm using the QD diameter and height as adjustable parameters. Assuming hole localization, this calculation yields values of Bm >20 T. The assumption that the hole localization diameter can be smaller than the QD diameter is justified due to alloy and spin disorder scattering. Using the magnetic polaron free energy, we calculate EMP as function of T and B for a variety of Bm values. To get a weak dependence of EMP on T and Bwe must assume that the polaron temperature is higher than T. This work was supported by U.S. DOE BES, Award DE-SC0004890, NSF DMR-1305770 and U.S. ONR N000141310754.
Quantum Magnetic Oscillations of the Surface Tension at a Metal-Insulator Interface
NASA Astrophysics Data System (ADS)
Dubovskii, L. B.
2016-03-01
Any metal-insulator transition (MI transition) in a crystalline material must be a transition from a situation in which electronic bands overlap to a situation when they do not (Mott, Metal-insulator, 2nd edn. Taylor@Francis, London, 1990). For this case the self-consistent equations for the two-band conductor are formulated (cf. Dubovskii, JETP Lett. 99(1):22-26, 2014). The description of the MI phase transition is based on two order parameters. The first one is the material density distribution at the MI boundary ρ ({vec {r}}). The second one is a four-component complex vector in spin space Upsilon ({vec {r}}). The value Upsilon ({vec {r}}) determines the electron density in the metallic or semimetallic phase in the presence of an external magnetic field. Two different components of the vector describe possible spin states of electrons and holes inserted in the external magnetic field. The solution gives a singular behavior of the surface tension at the MI interface in the vicinity of the MI phase transition. At low temperature quantum oscillations of the surface tension in the magnetic field take place.
Composite quantum spin liquid in a low-dimensional organometallic magnet
Stone, Matthew B; Tian, W.; Lumsden, Mark D; Granroth, Garrett E; Mandrus, David; Chung, J.-H.; Harrison, N.; Nagler, Stephen E
2007-01-01
The quantum magnet dimethylammonium trichlorocuprate (DMACuCl$_3$)has been considered an alternating antiferromagnetic-ferromagnetic (AFM-FM) chain along the $a$-axis, weakly coupled dimers along the $a$-axis and even a collection of isolated FM and AFM dimers. However, no spectroscopic probes have been applied until now to elucidate the underlying nature of the magnetic excitations. We present single crystal inelastic neutron scattering (INS) measurements that clearly indicate the magnetic excitations in DMACuCl$_3$ propagate along the $b$-axis. The spectrum has a gap $\\Delta = 0.95(2)$ meV and bandwidth of $0.71(2)$ meV with excitations characteristic of a quasi-1-dimensional alternating AFM-FM exchange chain. Values of exchange constants place DMACuCl$_3$ in a limit interpolating between coupled AFM $S=\\frac{1}{2}$ dimers and the $S=1$ Haldane chain. In order to consistently describe thermodynamic measurements with our spectroscopic results and the low-temperature crystal structure, we propose a composite two chain model where spin-spin interactions in one of the chains are very weakly correlated.
Urdampilleta, Matias; Nguyen, Ngoc-Viet; Cleuziou, Jean-Pierre; Klyatskaya, Svetlana; Ruben, Mario; Wernsdorfer, Wolfgang
2011-01-01
We built new hybrid devices consisting of chemical vapor deposition (CVD) grown carbon nanotube (CNT) transistors, decorated with TbPc(2) (Pc = phthalocyanine) rare-earth based single-molecule magnets (SMMs). The drafting was achieved by tailoring supramolecular π-π interactions between CNTs and SMMs. The magnetoresistance hysteresis loop measurements revealed steep steps, which we can relate to the magnetization reversal of individual SMMs. Indeed, we established that the electronic transport properties of these devices depend strongly on the relative magnetization orientations of the grafted SMMs. The SMMs are playing the role of localized spin polarizer and analyzer on the CNT electronic conducting channel. As a result, we measured magneto-resistance ratios up to several hundred percent. We used this spin valve effect to confirm the strong uniaxial anisotropy and the superparamagnetic blocking temperature (T(B) ~ 1 K) of isolated TbPc(2) SMMs. For the first time, the strength of exchange interaction between the different SMMs of the molecular spin valve geometry could be determined. Our results introduce a new design for operable molecular spintronic devices using the quantum effects of individual SMMs. PMID:22072910
Why a Magnetized Quantum Wire can Act as AN Optical Amplifier
NASA Astrophysics Data System (ADS)
Kushwaha, Manvir
We discuss the fundamental issues associated with the magnetoplasmon excitations in a semiconducting quantum wire characterized by a harmonic confining potential and subjected to an applied (perpendicular) magnetic field. The problem involves two length scales: l0 =√{ ℏ /m*ω0 } and lc =√{ ℏ /m*ωc } , which characterize the strengths of the confinement and the magnetic field (B). Essentially, we focus on the device aspects of the intersubband collective (magnetoroton) excitation, which observes a negative group velocity between maxon and roton. Existence of the negative group velocity is a clear manifestation of a medium with population inversion brought about due to a metastable state caused by the magnetic field that satisfies the condition B >Bth ; Bth being the threshold value below which the magnetoroton does not exist. A medium with an inverted population has the remarkable ability of amplifying a small optical signal of definite wavelength. An extensive scrutiny of the gain coefficient suggests an interesting and important application: the electronic device designed on the basis of such magnetoroton modes can act as an optical amplifier1.
Magnetism in parent Fe-chalcogenides: quantum fluctuations select a plaquette order
NASA Astrophysics Data System (ADS)
Perkins, Natalia; Ducatman, Samuel; Chubukov, Andrey
2013-03-01
The analysis of magnetism in parent compounds of iron-based superconductors (FeSCs) is an integral part of the program to understand the origin of superconductivity in these materials. Here we analyze magnetic order in iron-chalcogenide Fe1+yTe - the parent compound of high-temperature superconductor Fe1+yTe1-xSex. Neutron scattering experiments show that magnetic order in this material contains components with momentum Q1 = (π / 2 , π / 2) and Q2 = (π / 2 , - π / 2) in Fe-only Brillouin zone. The actual spin order depends on the interplay between these two components. Previous works argued that spin order is a single- Q state (either Q1 or Q2). Such an order breaks rotational C4 symmetry and order spins into a double diagonal stripe. We show that quantum fluctuations actually select another order - a double Q plaquette state with equal weight of Q1 and Q2 components, which preserves C4 symmetry but breaks Z4 translational symmetry. We argue that the plaquette state is consistent with recent neutron scattering experiments on Fe1+yTe. supported by the grant NSF-DMR-0844115
Unusual magnetic quantum oscillations in organic metals at high magnetic fields
Wosnitza, J.; Wanka, S.; Hagel, J.; Qualls, J. S.; Brooks, J. S.; Balthes, E.; Schweitzer, D.; Schlueter, J. A.; Geiser, U.
2000-04-04
The authors report on Shubnikov-de Haas (SdH) and de Haas-van Alphen (dHvA) results for the highly two-dimensional (2D) organic superconductors {kappa}-(ET){sub 2}I{sub 3} ({Tc} = 3.5 K) and {beta}{double_prime}-(ET){sub 2}SF{sub 5}CH{sub 2}CF{sub 2}SO{sub 3} ({Tc} = 4.4 K). The SdH oscillations of both materials show an apparent deviation from the well-understood 2D dHvA signal at low temperatures and high magnetic fields. For {kappa}-(ET){sub 2}I{sub 3}, the mechanism leading to this behavior still needs to be clarified. For {beta}{double_prime}-(ET){sub 2}SF{sub 5}CH{sub 2}CF{sub 2}SO{sub 3}, an anomalous steady background part of the magnetoresistance seems to account for the observed discrepancies.
NASA Astrophysics Data System (ADS)
Yakunin, M. V.; de Visser, Anne; Galistu, Gianni; Podgornykh, S. M.; Sadofyev, Yu G.; Shelushinina, N. G.; Harus, G. I.
2009-02-01
Development of quantum Hall peculiarities due to mobility gap between spin-split magnetic levels with addition of the parallel magnetic field component B|| is analyzed in double quantum wells (DQW) created in InGaAs/GaAs and InAs/AlSb heterosystems chosen due to their relatively large bulk g-factors. In InGaAs/GaAs DQWs, the nonmonotonous behavior of these peculiarities is observed and explained within single-electron approach in terms of competition between enhanced spin splitting and localization of electrons in the layers of DQW with increased B||. In InAs/AlSb DQW, the tunneling connection between the layers is very weak due to high barrier, nevertheless the collective odd-numbered peculiarities are revealed that exist due to spontaneous interlayer phase coherence. B|| destroys these states that is manifested, in particular, in the suppression of the peculiarity for filling factor v = 3.
Ferromagnetic ordered phase of quantum spin ice system Yb2Ti2O7 under [001] magnetic field
NASA Astrophysics Data System (ADS)
Hamachi, Noriaki; Yasui, Yukio; Araki, Koji; Kittaka, Shunichiro; Sakakibara, Toshiro
2016-05-01
Measurements of magnetization (M) and specific heat (C) under a [001] magnetic field were carried out on a single crystal of a quantum spin ice system Yb2Ti2O7 in order to investigate a feature of the transition occurred at TC ˜ 0.2 K. As a result of applying the magnetic field μ0H < 0.1 T, the C/T - T curve structure and transition temperature barely changed. On the other hand, applying the more than 0.1 T magnetic field, the C/T - T curve structure drastically change from sharp peak structure to broad peak one, and the broad peak temperature of C/T - T curves linearly increases with increasing magnetic field (H). In the magnetic field μ0H < 0.1 T, the magnetization drastically increases around TC ˜ 0.2 K with decreasing T, and a thermal hysteresis loop of the M - T curve is observed. With increasing H, the thermal hysteresis loop of the M - T curves disappears above μ0HC = 0.1 T. We can understand these results, where Yb2Ti2O7 exhibits a first-order ferromagnetic transition associated with the latent heat corresponding to the energy of μ0HC = 0.1 T. Basis of the H - T phase diagram along [001] magnetic field, the feature of the transition occurred at TC ˜ 0.2 K in quantum spin ice system Yb2Ti2O7 is discussed.
Magneto-transport studies of a few hole GaAs double quantum dot in tilted magnetic fields
NASA Astrophysics Data System (ADS)
Studenikin, Sergei; Bogan, Alex; Tracy, Lisa; Gaudreau, Louis; Sachrajda, Andy; Korkusinski, Marek; Reno, John; Hargett, Terry
Compared to equivalent electron devices, single-hole spins interact weakly with lattice nuclear spins leading to extended quantum coherence times. This makes p-type Quantum Dots (QD) particularly attractive for practical quantum devices such as qubit circuits, quantum repeaters, quantum sensors etc. where long coherence time is required. Another property of holes is the possibility to tune their g-factor as a result of the strong anisotropy of the valance band. Hole g-factors can be conveniently tuned in situ from a large value to almost zero by tilting the magnetic field relative to the 2D hole gas surface normal. In this work we explore high-bias magneto-transport properties of a p-type double quantum dot (DQD) device fabricated from a GaAs/AlGaAs heterostructures using lateral split-gate technology. A charge detection technique is used to monitor number of holes and tune the p-DQD in a single hole regime around (1,1) and (2,0) occupation states where Pauli spin-blockaded transport is expected. Four states are identified in quantizing magnetic fields within the high-bias current stripe - three-fold triplet and a singlet which allows determining effective heavy hole g-factor as a function of the tilt angle from 90 to 0 degrees.
Magnetic field dependent photoluminescence studies of InGaAs/GaAs strained-single-quantum wells
Jones, E.D.; Dawson, L.R.; Klem, J.F.; Lyo, S.K.; Heiman, D.; Liu, X.C.
1994-08-01
Magnetoluminescence determined conduction-band and valence-band dispersion curves are presented for n-type InGaAs/GaAs stained-single-quantum well structures. The magnetic field range was 0 to 30 tesla, and the temperature varied between 4.2 and 77.4 K.
Falaye, Babatunde James; Sun, Guo-Hua; Silva-Ortigoza, Ramón; Dong, Shi-Hai
2016-05-01
This study presents the confinement influences of Aharonov-Bohm (AB) flux and electric and magnetic fields directed along the z axis and encircled by quantum plasmas on the hydrogen atom. The all-inclusive effects result in a strongly attractive system while the localizations of quantum levels change and the eigenvalues decrease. We find that the combined effect of the fields is stronger than a solitary effect and consequently there is a substantial shift in the bound state energy of the system. We also find that to perpetuate a low-energy medium for the hydrogen atom in quantum plasmas, a strong electric field and weak magnetic field are required, whereas the AB flux field can be used as a regulator. The application of the perturbation technique utilized in this paper is not restricted to plasma physics; it can also be applied in molecular physics. PMID:27300989
NASA Astrophysics Data System (ADS)
Falaye, Babatunde James; Sun, Guo-Hua; Silva-Ortigoza, Ramón; Dong, Shi-Hai
2016-05-01
This study presents the confinement influences of Aharonov-Bohm (AB) flux and electric and magnetic fields directed along the z axis and encircled by quantum plasmas on the hydrogen atom. The all-inclusive effects result in a strongly attractive system while the localizations of quantum levels change and the eigenvalues decrease. We find that the combined effect of the fields is stronger than a solitary effect and consequently there is a substantial shift in the bound state energy of the system. We also find that to perpetuate a low-energy medium for the hydrogen atom in quantum plasmas, a strong electric field and weak magnetic field are required, whereas the AB flux field can be used as a regulator. The application of the perturbation technique utilized in this paper is not restricted to plasma physics; it can also be applied in molecular physics.
Magnetic field induced indirect gap in a modulation doped quantum well
NASA Astrophysics Data System (ADS)
Whittaker, D. M.; Fisher, T. A.; Simmonds, P. E.; Skolnick, M. S.; Smith, R. S.; Taylor, L. L.; Bass, S. J.
1992-02-01
We report the first experimental evidence for the indirect fundamental band-gap developed when an in-plane magnetic field is applied to a wide, modulation-doped quantum well. In such structures, band bending may cause the lowest energy electron and hole states to be spatially separated, which leads to an induced indirect gap proportional to the field. The corresponding photoluminescence peak undergoes a large, roughly quadratic shift with field, a consequence of the behaviour of the allowed transitions involving thermalised holes and electrons with finite k. This characteristic strong diamagnetic shift is observed in spectra from both asymmetric AlGaAs/InGaAs/GaAs strained layer structures and a very wide symmetric InGaAs/InP lattice matched well. The experimental results are shown to be in good agreement with realistic self consistent calculations of the band-structure.
Itinerancy enhanced quantum fluctuation of magnetic moments in iron-based superconductors
Tam, Yu -T.; Ku, W.; Yao, D. -X.
2015-09-10
We investigate the influence of itinerant carriers on dynamics and fluctuation of local moments in Fe-based superconductors, via linear spin-wave analysis of a spin-fermion model containing both itinerant and local degrees of freedom. Surprisingly against the common lore, instead of enhancing the (π,0) order, itinerant carriers with well nested Fermi surfaces is found to induce significant amount of spatial and temporal quantum fluctuation that leads to the observed small ordered moment. Interestingly, the underlying mechanism is shown to be intra-pocket nesting-associated long-range coupling, rather than the previously believed ferromagnetic double-exchange effect. This challenges the validity of ferromagnetically compensated first-neighbor couplingmore » reported from short-range fitting to the experimental dispersion, which turns out to result instead from the ferro-orbital order that is also found instrumental in stabilizing the magnetic order.« less
Itinerancy enhanced quantum fluctuation of magnetic moments in iron-based superconductors
Tam, Yu -T.; Ku, W.; Yao, D. -X.
2015-09-10
We investigate the influence of itinerant carriers on dynamics and fluctuation of local moments in Fe-based superconductors, via linear spin-wave analysis of a spin-fermion model containing both itinerant and local degrees of freedom. Surprisingly against the common lore, instead of enhancing the (π,0) order, itinerant carriers with well nested Fermi surfaces is found to induce significant amount of spatial and temporal quantum fluctuation that leads to the observed small ordered moment. Interestingly, the underlying mechanism is shown to be intra-pocket nesting-associated long-range coupling, rather than the previously believed ferromagnetic double-exchange effect. This challenges the validity of ferromagnetically compensated first-neighbor coupling reported from short-range fitting to the experimental dispersion, which turns out to result instead from the ferro-orbital order that is also found instrumental in stabilizing the magnetic order.
Park, Hoyoung; Lee, Jong-Wook; Hwang, Mintai P; Lee, Kwan Hyi
2013-09-21
Cardiovascular disease (CVD) is a potent cause of mortality in both advanced and developing countries. While soluble CD40L (sCD40L) has been implicated as a correlative factor among CVD patients, methods to quantify sCD40L are not yet well-established. In this paper, we present an ability to separate and quantify sCD40L via a simple immunomagnetic assay. Composed of functionalized magnetic beads conferred with directionality and on-demand detachable quantum dots for subsequent optical analysis, our system utilizes the competitive nature of imidazole and nickel ions for histidine. In essence, we demonstrate the capacity to effectively separate and detect sCD40L within a clinically relevant range that contains the cut-off value for acute coronary disease. While sCD40L was used to conduct this study, we envision the use of our system for the separation and quantification of other biomarkers. PMID:23893124
Three-Dimensional Crystallization of Vortex Strings in Frustrated Quantum Magnets
NASA Astrophysics Data System (ADS)
Wang, Zhentao; Kamiya, Yoshitomo; Nevidomskyy, Andriy H.; Batista, Cristian D.
2015-09-01
We demonstrate that frustrated exchange interactions can produce exotic 3D crystals of vortex strings near the saturation field (H =Hsat) of body- and face-centered cubic Mott insulators. The combination of cubic symmetry and frustration leads to a magnon spectrum of the fully polarized spin state (H >Hsat) with degenerate minima at multiple noncoplanar Q vectors. This spectrum becomes gapless at the quantum critical point H =Hsat and the magnetic ordering below Hsat can be formally described as a condensate of a dilute gas of bosons. By expanding in the lattice gas parameter, we find that different vortex crystals span sizable regions of the phase diagrams for isotropic exchange and are further stabilized by symmetric exchange anisotropy.
NASA Astrophysics Data System (ADS)
Park, Hoyoung; Lee, Jong-Wook; Hwang, Mintai P.; Lee, Kwan Hyi
2013-08-01
Cardiovascular disease (CVD) is a potent cause of mortality in both advanced and developing countries. While soluble CD40L (sCD40L) has been implicated as a correlative factor among CVD patients, methods to quantify sCD40L are not yet well-established. In this paper, we present an ability to separate and quantify sCD40L via a simple immunomagnetic assay. Composed of functionalized magnetic beads conferred with directionality and on-demand detachable quantum dots for subsequent optical analysis, our system utilizes the competitive nature of imidazole and nickel ions for histidine. In essence, we demonstrate the capacity to effectively separate and detect sCD40L within a clinically relevant range that contains the cut-off value for acute coronary disease. While sCD40L was used to conduct this study, we envision the use of our system for the separation and quantification of other biomarkers.
Itinerancy-enhanced quantum fluctuation of magnetic moments in iron-based superconductors.
Tam, Yu-Ting; Yao, Dao-Xin; Ku, Wei
2015-09-11
We investigate the influence of itinerant carriers on the dynamics and fluctuation of local moments in Fe-based superconductors, via linear spin-wave analysis of a spin-fermion model containing both itinerant and local degrees of freedom. Surprisingly, against the common lore, instead of enhancing the (π,0) order, itinerant carriers with well-nested Fermi surfaces are found to induce a significant amount of spatial and temporal quantum fluctuation that leads to the observed small ordered moment. Interestingly, the underlying mechanism is shown to be an intrapocket nesting-associated long-range coupling rather than the previously believed ferromagnetic double-exchange effect. This challenges the validity of ferromagnetically compensated first-neighbor coupling reported from short-range fitting to the experimental dispersion, which turns out to result instead from the ferro-orbital order that is also found instrumental in stabilizing the magnetic order. PMID:26406850
Itinerancy-Enhanced Quantum Fluctuation of Magnetic Moments in Iron-Based Superconductors
NASA Astrophysics Data System (ADS)
Tam, Yu-Ting; Yao, Dao-Xin; Ku, Wei
2015-09-01
We investigate the influence of itinerant carriers on the dynamics and fluctuation of local moments in Fe-based superconductors, via linear spin-wave analysis of a spin-fermion model containing both itinerant and local degrees of freedom. Surprisingly, against the common lore, instead of enhancing the (π ,0 ) order, itinerant carriers with well-nested Fermi surfaces are found to induce a significant amount of spatial and temporal quantum fluctuation that leads to the observed small ordered moment. Interestingly, the underlying mechanism is shown to be an intrapocket nesting-associated long-range coupling rather than the previously believed ferromagnetic double-exchange effect. This challenges the validity of ferromagnetically compensated first-neighbor coupling reported from short-range fitting to the experimental dispersion, which turns out to result instead from the ferro-orbital order that is also found instrumental in stabilizing the magnetic order.
Three-Dimensional Crystallization of Vortex Strings in Frustrated Quantum Magnets.
Wang, Zhentao; Kamiya, Yoshitomo; Nevidomskyy, Andriy H; Batista, Cristian D
2015-09-01
We demonstrate that frustrated exchange interactions can produce exotic 3D crystals of vortex strings near the saturation field (H=H(sat)) of body- and face-centered cubic Mott insulators. The combination of cubic symmetry and frustration leads to a magnon spectrum of the fully polarized spin state (H>H(sat)) with degenerate minima at multiple noncoplanar Q vectors. This spectrum becomes gapless at the quantum critical point H=H(sat) and the magnetic ordering below H(sat) can be formally described as a condensate of a dilute gas of bosons. By expanding in the lattice gas parameter, we find that different vortex crystals span sizable regions of the phase diagrams for isotropic exchange and are further stabilized by symmetric exchange anisotropy. PMID:26382699
Miller, D.; Milton, K.A.; Siegemund-Broka, S. )
1992-07-15
This is the first in a series of papers dealing with four-dimensional quantum electrodynamics on a finite-element lattice. We begin by studying the canonical structure of the theory without interactions. This tells us how to construct momentum expansions for the field operators. Next we examine the interaction term in the Dirac equation. We construct the transfer matrix explicitly in the temporal gauge, and show that it is unitary. Therefore, fermion canonical anticommutation relations hold at each lattice site. Finally, we expand the interaction term to second order in the temporal-lattice spacing and deduce the magnetic moment of the electron in a background field, consistent with the continuum value of {ital g}=2.
Luminescence of double quantum wells subject to in-plane magnetic fields
NASA Astrophysics Data System (ADS)
Orlita, M.; Grill, R.; Hlídek, P.; Zvára, M.; Döhler, G. H.; Malzer, S.; Byszewski, M.
2005-10-01
We report on photoluminescence (PL) measurements of a symmetric GaAs/AlGaAs double quantum well (DQW) in high magnetic fields. For this study, a selectively contacted p-δn-DQW-δn-p structure was chosen, allowing an independent tuning of the electron density in the DQW and thus a creation of a two-dimensional electron gas. Our attention was focused on phenomena in in-plane magnetic fields, where the field-induced depopulation of the antibonding subband observable in the PL spectra as a so-called N -type kink was predicted by Huang and Lyo (HL) [Phys. Rev. B 59, 7600 (1999)]. Whereas the equivalent behavior has been observed several times in the electric transport measurements and a proper theoretical description has been found, to the best of our knowledge, no PL experiment in a direct comparison with the theoretical model developed by HL has ever been published. We carried out a self-consistent calculation based on their model and achieved a good agreement with our experimental results. Additionally, the influence of the excitonic interaction on the PL spectra, not taken into account by HL, is also discussed. This enables us to explain small deviations from the HL theory. The interpretation of the in-plane magnetic field measurements is supported by the experiment with the magnetic field in the perpendicular orientation that allows a sufficiently accurate estimation of the electron density in the DQW. Distinctive renormalization effects of DQW subbands at various electron densities are also observed and discussed.
Pervishko, A A; Kibis, O V; Shelykh, I A
2016-08-01
We investigate theoretically the effect of a magnetic field on intersubband polaritons in an asymmetric quantum well placed inside an optical resonator. It is demonstrated that the field-induced diamagnetic shift of electron subbands in the well increases the broadening of optical lines corresponding to intersubband electron transitions. As a consequence, the magnetic field can switch the polariton system from the regime of strong light-matter coupling to the regime of a weak one. This effect paves a way for the effective control of polaritonic devices with a magnetic field. PMID:27472627
NASA Astrophysics Data System (ADS)
Pervishko, A. A.; Kibis, O. V.; Shelykh, I. A.
2016-08-01
We investigate theoretically the effect of a magnetic field on intersubband polaritons in an asymmetric quantum well placed inside an optical resonator. It is demonstrated that the field-induced diamagnetic shift of electron subbands in the well increases the broadening of optical lines corresponding to intersubband electron transitions. As a consequence, the magnetic field can switch the polariton system from the regime of strong light-matter coupling to the regime of weak one. This effect paves a way to the effective control of polaritonic devices with a magnetic field.
Zhang, Xi; Wang, Chao; Diao, Dongfeng; Sun, Chang Q
2014-07-28
In this paper, we clarified a robust mechanism of magnetism generated by excess electrons captured by edge-quantum well of diamagnetic armchair edges. Consistency between density functional theory calculations and electron cyclotron resonance experiments verified that: (1) Multi-layer armchair nanoribbons are stable with proper amounts of excess electrons which can provide net spin; (2) Since under-coordination induces lattice relaxation and potential well modulation, electrons tend to be trapped at edges; and (3) Neither large amount of excess electrons nor positive charges can induce magnetism. This work shed light on the development of graphene devices in its magnetic applications.
NASA Astrophysics Data System (ADS)
B, Gisi; S, Sakiroglu; İ, Sokmen
2016-01-01
In this work, we investigate the effects of interplay of spin-orbit interaction and in-plane magnetic fields on the electronic structure and spin texturing of parabolically confined quantum wire. Numerical results reveal that the competing effects between Rashba and Dresselhaus spin-orbit interactions and the external magnetic field lead to a complicated energy spectrum. We find that the spin texturing owing to the coupling between subbands can be modified by the strength of spin-orbit couplings as well as the magnitude and the orientation angle of the external magnetic field.
Quantum magnetism in strongly interacting one-dimensional spinor Bose systems
Dehkharghani, Amin; Volosniev, Artem; Lindgren, Jonathan; Rotureau, Jimmy; Forssén, Christian; Fedorov, Dmitri; Jensen, Aksel; Zinner, Nikolaj
2015-01-01
Strongly interacting one-dimensional quantum systems often behave in a manner that is distinctly different from their higher-dimensional counterparts. When a particle attempts to move in a one-dimensional environment it will unavoidably have to interact and ‘push’ other particles in order to execute a pattern of motion, irrespective of whether the particles are fermions or bosons. A present frontier in both theory and experiment are mixed systems of different species and/or particles with multiple internal degrees of freedom. Here we consider trapped two-component bosons with short-range inter-species interactions much larger than their intra-species interactions and show that they have novel energetic and magnetic properties. In the strongly interacting regime, these systems have energies that are fractions of the basic harmonic oscillator trap quantum and have spatially separated ground states with manifestly ferromagnetic wave functions. Furthermore, we predict excited states that have perfect antiferromagnetic ordering. This holds for both balanced and imbalanced systems, and we show that it is a generic feature as one crosses from few- to many-body systems. PMID:26073680