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Sample records for pure spin states

  1. Quantum well state induced oscillation of pure spin currents in Fe/Au/Pd(001) systems.

    PubMed

    Montoya, Eric; Heinrich, Bret; Girt, Erol

    2014-09-26

    Spin pumping at the ferromagnetic metal (Fe)/normal metal (Au) interface and the subsequent spin transport in Au/Pd heterostructures is studied using ferromagnetic resonance. The spin pumping induced damping in the Fe/Pd structure is greatly suppressed by the addition of a Au spacer layer in the structure Fe/Au/Pd. The rapid decrease in the interface damping with an increasing Au layer thickness does not correspond to an expectation based on a simple spin diffusion theory in the Au layer. It is possible to account for this behavior by introducing a partial reflection of spin current at the Au/Pd interface. Furthermore, oscillations in the amplitude of spin pumping damping are observed in the Fe/Au/Pd structure as a function of Au thickness for thicknesses less than half the electron mean free path of bulk Au. This new effect indicates a formation of quantum well states in the accumulated spin density in the Au spacer that affect the time irreversible process of spin pumping. PMID:25302912

  2. Canonical Thermal Pure Quantum State

    NASA Astrophysics Data System (ADS)

    Sugiura, Sho; Shimizu, Akira

    2013-07-01

    A thermal equilibrium state of a quantum many-body system can be represented by a typical pure state, which we call a thermal pure quantum (TPQ) state. We construct the canonical TPQ state, which corresponds to the canonical ensemble of the conventional statistical mechanics. It is related to the microcanonical TPQ state, which corresponds to the microcanonical ensemble, by simple analytic transformations. Both TPQ states give identical thermodynamic results, if both ensembles do, in the thermodynamic limit. The TPQ states corresponding to other ensembles can also be constructed. We have thus established the TPQ formulation of statistical mechanics, according to which all quantities of statistical-mechanical interest are obtained from a single realization of any TPQ state. We also show that it has great advantages in practical applications. As an illustration, we study the spin-1/2 kagome Heisenberg antiferromagnet.

  3. Pure quantum dephasing of a solid-state electron spin qubit in a large nuclear spin bath coupled by long-range hyperfine-mediated interactions

    NASA Astrophysics Data System (ADS)

    Cywiński, Łukasz; Witzel, Wayne M.; Das Sarma, S.

    2009-06-01

    We investigate decoherence due to pure dephasing of a localized spin qubit interacting with a nuclear spin bath. Although in the limit of a very large magnetic field the only decoherence mechanism is spectral diffusion due to dipolar flip-flops of nuclear spins, with decreasing field the hyperfine-mediated interactions between the nuclear spins become important. We take advantage of their long-range nature and resum the leading terms in an 1/N expansion of the decoherence time-evolution function ( N , being the number of nuclear spins interacting appreciably with the electron spin, is large). For the case of the thermal uncorrelated bath we show that our theory is applicable down to low magnetic fields ( ˜10mT for a large dot with N=106 ) allowing for comparison with recent experiments in GaAs quantum dot spin qubits. Within this approach we calculate the free induction decay and spin echo decoherence in GaAs and InGaAs as a function of the number of the nuclei in the bath (i.e., the quantum dot size) and the magnetic field. Our theory for free induction decay in a narrowed nuclear bath is shown to agree with the exact solution for decoherence due to hyperfine-mediated interaction which can be obtained when all the nuclei-electron coupling constants are identical. For the spin echo evolution we show that the dominant decoherence process at low fields is due to interactions between nuclei having significantly different Zeeman energies (i.e., nuclei of As and two isotopes of Ga in GaAs), and we compare our results with recent measurements of spin echo signal of a single spin confined in a GaAs quantum dot. For the same set of parameters we perform calculations of decoherence under various dynamical decoupling pulse sequences and predict the effect of these sequences in low- B regime in GaAs.

  4. Excitation of coherent propagating spin waves by pure spin currents

    NASA Astrophysics Data System (ADS)

    Demidov, Vladislav E.; Urazhdin, Sergei; Liu, Ronghua; Divinskiy, Boris; Telegin, Andrey; Demokritov, Sergej O.

    2016-01-01

    Utilization of pure spin currents not accompanied by the flow of electrical charge provides unprecedented opportunities for the emerging technologies based on the electron's spin degree of freedom, such as spintronics and magnonics. It was recently shown that pure spin currents can be used to excite coherent magnetization dynamics in magnetic nanostructures. However, because of the intrinsic nonlinear self-localization effects, magnetic auto-oscillations in the demonstrated devices were spatially confined, preventing their applications as sources of propagating spin waves in magnonic circuits using these waves as signal carriers. Here, we experimentally demonstrate efficient excitation and directional propagation of coherent spin waves generated by pure spin current. We show that this can be achieved by using the nonlocal spin injection mechanism, which enables flexible design of magnetic nanosystems and allows one to efficiently control their dynamic characteristics.

  5. Excitation of coherent propagating spin waves by pure spin currents.

    PubMed

    Demidov, Vladislav E; Urazhdin, Sergei; Liu, Ronghua; Divinskiy, Boris; Telegin, Andrey; Demokritov, Sergej O

    2016-01-01

    Utilization of pure spin currents not accompanied by the flow of electrical charge provides unprecedented opportunities for the emerging technologies based on the electron's spin degree of freedom, such as spintronics and magnonics. It was recently shown that pure spin currents can be used to excite coherent magnetization dynamics in magnetic nanostructures. However, because of the intrinsic nonlinear self-localization effects, magnetic auto-oscillations in the demonstrated devices were spatially confined, preventing their applications as sources of propagating spin waves in magnonic circuits using these waves as signal carriers. Here, we experimentally demonstrate efficient excitation and directional propagation of coherent spin waves generated by pure spin current. We show that this can be achieved by using the nonlocal spin injection mechanism, which enables flexible design of magnetic nanosystems and allows one to efficiently control their dynamic characteristics. PMID:26818232

  6. Excitation of coherent propagating spin waves by pure spin currents

    PubMed Central

    Demidov, Vladislav E.; Urazhdin, Sergei; Liu, Ronghua; Divinskiy, Boris; Telegin, Andrey; Demokritov, Sergej O.

    2016-01-01

    Utilization of pure spin currents not accompanied by the flow of electrical charge provides unprecedented opportunities for the emerging technologies based on the electron's spin degree of freedom, such as spintronics and magnonics. It was recently shown that pure spin currents can be used to excite coherent magnetization dynamics in magnetic nanostructures. However, because of the intrinsic nonlinear self-localization effects, magnetic auto-oscillations in the demonstrated devices were spatially confined, preventing their applications as sources of propagating spin waves in magnonic circuits using these waves as signal carriers. Here, we experimentally demonstrate efficient excitation and directional propagation of coherent spin waves generated by pure spin current. We show that this can be achieved by using the nonlocal spin injection mechanism, which enables flexible design of magnetic nanosystems and allows one to efficiently control their dynamic characteristics. PMID:26818232

  7. Direct measurement of the concurrence for two-qubit electron spin entangled pure state based on charge detection

    NASA Astrophysics Data System (ADS)

    Liu, Jiong; Zhou, Lan; Sheng, Yu-Bo

    2015-07-01

    We propose a protocol for directly measuring the concurrence of a two-qubit electronic pure entangled state. To complete this task, we first design a parity-check measurement (PCM) which is constructed by two polarization beam splitters (PBSs) and a charge detector. By using the PCM for three rounds, we can achieve the concurrence by calculating the total probability of picking up the odd parity states from the initial states. Since the conduction electron may be a good candidate for the realization of quantum computation, this protocol may be useful in future solid quantum computation. Project supported by the National Natural Science Foundation of China (Grant Nos. 11474168 and 61401222), the Qing Lan Project in Jiangsu Province, China, and the Priority Academic Development Program of Jiangsu Higher Education Institutions, China.

  8. Quantumness of spin-1 states

    NASA Astrophysics Data System (ADS)

    Bohnet-Waldraff, Fabian; Braun, D.; Giraud, O.

    2016-01-01

    We investigate quantumness of spin-1 states, defined as the Hilbert-Schmidt distance to the convex hull of spin coherent states. We derive its analytic expression in the case of pure states as a function of the smallest eigenvalue of the Bloch matrix and give explicitly the closest classical state for an arbitrary pure state. Numerical evidence is given that the exact formula for pure states provides an upper bound on the quantumness of mixed states. Due to the connection between quantumness and entanglement we obtain new insights into the geometry of symmetric entangled states.

  9. Pure spin current in lateral structures

    NASA Astrophysics Data System (ADS)

    Chen, Shuhan

    Spintronics, a frontier academic research area, is advancing rapidly in recent years. It has been chosen as one of the promising candidates for overcoming the obstacles in continuing the "Moore's Law" of the electronics industry. Spintronics employs both spin and charge degrees of freedom of electrons to reduce energy consumption and increase the flexibility of IC design. To achieve this, it is extremely important to understand the generation, transport, and detection of the spin polarized current (spin current). In this work we use a mesoscopic metallic spintronic structure-nonlocal spin valve (NLSV)-for fundamental studies of spintronics. A nonlocal spin valve consists of two ferromagnetic electrodes (a spin injector and a spin detector) bridged by a non-magnetic spin channel. A thin aluminum oxide barrier (~ 2 - 3 nm) has been shown to effectively enhance the spin injection and detection polarizations. We have studied spin injection and detection in these nanoscale structures. Several topics will be discussed in this work. In Chapter 4 we explore spin transport in NLSVs with Ag channels. Substantial spin signals are observed. The temperature dependence of the spin signals indicates long spin diffusion lengths and low surface spin-flip rate in the mesoscopic Ag channels. Chapter 5 will focus on the asymmetric spin absorption across the low-resistance AlOx barriers in NLSVs. This effect allows for a more simplified and efficient detection scheme for the spin accumulation. Then in Chapter 6 we report a large spin signal owing to a highly resistive break-junction. We have also developed a model to describe the spin-charge coupling effect which enables the large spin signal. In the end, Spin Hall Effect (SHE) is investigated in Chapter 7. A mesoscopic Pt film is utilized to inject a spin accumulation into a mesoscopic Cu channel via the SHE. The spin accumulation in Cu can be detected by the nonlocal method. The reciprocal effect -- the inverse Spin Hall Effect - (i

  10. Anisotropic Absorption of Pure Spin Currents

    NASA Astrophysics Data System (ADS)

    Baker, A. A.; Figueroa, A. I.; Love, C. J.; Cavill, S. A.; Hesjedal, T.; van der Laan, G.

    2016-01-01

    Spin transfer in magnetic multilayers offers the possibility of ultrafast, low-power device operation. We report a study of spin pumping in spin valves, demonstrating that a strong anisotropy of spin pumping from the source layer can be induced by an angular dependence of the total Gilbert damping parameter, α , in the spin sink layer. Using lab- and synchrotron-based ferromagnetic resonance, we show that an in-plane variation of damping in a crystalline Co50 Fe50 layer leads to an anisotropic α in a polycrystalline Ni81 Fe19 layer. This anisotropy is suppressed above the spin diffusion length in Cr, which is found to be 8 nm, and is independent of static exchange coupling in the spin valve. These results offer a valuable insight into the transmission and absorption of spin currents, and a mechanism by which enhanced spin torques and angular control may be realized for next-generation spintronic devices.

  11. Anisotropic Absorption of Pure Spin Currents.

    PubMed

    Baker, A A; Figueroa, A I; Love, C J; Cavill, S A; Hesjedal, T; van der Laan, G

    2016-01-29

    Spin transfer in magnetic multilayers offers the possibility of ultrafast, low-power device operation. We report a study of spin pumping in spin valves, demonstrating that a strong anisotropy of spin pumping from the source layer can be induced by an angular dependence of the total Gilbert damping parameter, α, in the spin sink layer. Using lab- and synchrotron-based ferromagnetic resonance, we show that an in-plane variation of damping in a crystalline Co_{50}Fe_{50} layer leads to an anisotropic α in a polycrystalline Ni_{81}Fe_{19} layer. This anisotropy is suppressed above the spin diffusion length in Cr, which is found to be 8 nm, and is independent of static exchange coupling in the spin valve. These results offer a valuable insight into the transmission and absorption of spin currents, and a mechanism by which enhanced spin torques and angular control may be realized for next-generation spintronic devices. PMID:26871353

  12. Ultrahigh spin thermopower and pure spin current in a single-molecule magnet

    PubMed Central

    Luo, Bo; Liu, Juan; Lü, Jing-Tao; Gao, Jin-Hua; Yao, Kai-Lun

    2014-01-01

    Using the non-equilibrium Green's function (NEGF) formalism within the sequential regime, we studied ultrahigh spin thermopower and pure spin current in single-molecule magnet(SMM), which is attached to nonmagnetic metal wires with spin bias and angle (θ) between the easy axis of SMM and the spin orientation in the electrodes. A pure spin current can be generated by tuning the gate voltage and temperature difference with finite spin bias and the arbitrary angle except of . In the linear regime, large thermopower can be obtained by modifying Vg and the angles (θ). These results are useful in fabricating and advantaging SMM devices based on spin caloritronics. PMID:24549224

  13. Demonstration of Kirchhoff's First Law for Pure Spin Currents

    NASA Astrophysics Data System (ADS)

    Batley, Joseph; Rosamond, M. C.; Ali, M.; Linfield, E. H.; Burnell, G.; Hickey, B. J.

    In conventional electronics a fundamental component of circuit design is the principle of fan-out, which allows multiple operations to be performed in order to build up complex logical procedures. A fan-out device relies on the condition that electrical currents obey Kirchoff's laws and in order for spin-logic to be viable, the same must be shown for pure spin currents. Both fan-out and fan-in experiments have been performed to observe how spin currents behave in a multi-terminal circuit. The development of a 3-dimensional nonlocal IV and matrix fitting method provides information about each spin current, along with the thermal current generated at the injection point, and how they interact with each other. The fan-out geometry demonstrates that a pure spin current will divide between the different branches in a circuit, with a magnitude determined through the spin resistances of each arm. The fan-in measurements demonstrate that two pure spin currents will add and subtract with each other in a conventional manner expected from Kirchhoff's first law. These experiments have demonstrated the symmetry of pure spin currents with respect to the injection current and shown that they obey Kirchhoff's current law.

  14. Heat production by diffusion of pure spin current

    NASA Astrophysics Data System (ADS)

    Taniguchi, Tomohiro; Saslow, Wayne M.

    2016-02-01

    The theoretical investigation of the dissipation due to a pure spin current generated by spin pumping in a ferromagnetic/nonmagnetic bilayer is studied. The analytical solution of the dissipation is specifically derived. We show that the dissipation becomes zero when the spin diffusion length of the nonmagnet becomes sufficiently longer than its thickness. We also show that the second law of the thermodynamics is guaranteed.

  15. Mixtures of maximally entangled pure states

    NASA Astrophysics Data System (ADS)

    Flores, M. M.; Galapon, E. A.

    2016-09-01

    We study the conditions when mixtures of maximally entangled pure states remain entangled. We found that the resulting mixed state remains entangled when the number of entangled pure states to be mixed is less than or equal to the dimension of the pure states. For the latter case of mixing a number of pure states equal to their dimension, we found that the mixed state is entangled provided that the entangled pure states to be mixed are not equally weighted. We also found that one can restrict the set of pure states that one can mix from in order to ensure that the resulting mixed state is genuinely entangled. Also, we demonstrate how these results could be applied as a way to detect entanglement in mixtures of the entangled pure states with noise.

  16. A measurement of. Delta. sigma. sub L (np), the difference between neutron-proton total cross sections in pure longitudinal spin states

    SciTech Connect

    Beddo, M.E.

    1990-10-01

    A measurement off {Delta}{sigma}{sub L}(np), the difference between neutron-proton total cross sections in pure longitudinal spin states, is described. The results will help determine the isospin-zero (I = 0) scattering amplitudes, which are not well known above laboratory energies of 500 MeV, whereas the isospin-one (I = 1) amplitudes are fairly well-determined to 1 GeV. Data points were taken at the Los Alamos Meson Physics Facility (LAMPF) at Los Alamos, New Mexico, for five neutron beam energies: 484, 568, 634,720 and 788 MeV; they are the first in this energy range. Polarized neutrons were produced by charge-exchange of polarized protons on a liquid deuterium target (LD{sub 2}). Large-volume neutron counters detected the neutrons that passed through a polarized proton target. The counters subtended a range of solid angles large enough to allow extrapolation of the scattered neutrons to 0{degree}. Two modifications to the LAMPF accelerator system which were made for this work are described. They included a beam buncher,'' which modified the normal rf-time structure of the proton beam and allowed for the selection of peak-energy neutrons by time-of-flight means, and a computerized beam steering program, which reduced systematic effects due to beam motion at the LD{sub 2} target. The experimental values of {Delta}{sigma}{sub L}(np) are found to be consistent with other np data, including preliminary data from SIN and Saclay, but not with some results from Argonne which used a polarized proton beam and a polarized deuteron target. The I = 0 component was extracted from {Delta}{sigma}{sub L}(np) using existing pp data (I = 1), with the unexpected result that {Delta}{sigma}{sub L}(I = 0) was found to be essentially identical in shape to {Delta}{sigma}{sub L}(I = 1). The significance of this is not yet understood.

  17. Modulation of pure spin currents with a ferromagnetic insulator

    NASA Astrophysics Data System (ADS)

    Villamor, Estitxu; Isasa, Miren; Vélez, Saül; Bedoya-Pinto, Amilcar; Vavassori, Paolo; Hueso, Luis E.; Bergeret, F. Sebastián; Casanova, Fèlix

    2015-01-01

    We propose and demonstrate spin manipulation by magnetically controlled modulation of pure spin currents in cobalt/copper lateral spin valves, fabricated on top of the magnetic insulator Y3F e5O12 (YIG). The direction of the YIG magnetization can be controlled by a small magnetic field. We observe a clear modulation of the nonlocal resistance as a function of the orientation of the YIG magnetization with respect to the polarization of the spin current. Such a modulation can only be explained by assuming a finite spin-mixing conductance at the Cu/YIG interface, as it follows from the solution of the spin-diffusion equation. These results open a path towards the development of spin logics.

  18. Magnetic nano-oscillator driven by pure spin current

    NASA Astrophysics Data System (ADS)

    Demidov, Vladislav E.; Urazhdin, Sergei; Ulrichs, Henning; Tiberkevich, Vasyl; Slavin, Andrei; Baither, Dietmar; Schmitz, Guido; Demokritov, Sergej O.

    2012-12-01

    With the advent of pure-spin-current sources, spin-based electronic (spintronic) devices no longer require electrical charge transfer, opening new possibilities for both conducting and insulating spintronic systems. Pure spin currents have been used to suppress noise caused by thermal fluctuations in magnetic nanodevices, amplify propagating magnetization waves, and to reduce the dynamic damping in magnetic films. However, generation of coherent auto-oscillations by pure spin currents has not been achieved so far. Here we demonstrate the generation of single-mode coherent auto-oscillations in a device that combines local injection of a pure spin current with enhanced spin-wave radiation losses. Counterintuitively, radiation losses enable excitation of auto-oscillation, suppressing the nonlinear processes that prevent auto-oscillation by redistributing the energy between different modes. Our devices exhibit auto-oscillations at moderate current densities, at a microwave frequency tunable over a wide range. These findings suggest a new route for the implementation of nanoscale microwave sources for next-generation integrated electronics.

  19. Excitations of the spin-density wave in pure chromium

    SciTech Connect

    Werner, S.A.; Shirane, G.; Fincher, C.R.; Grier, B.H.

    1981-01-01

    This paper summarizes recent investigations of the magnetic excitations of the spin density wave (SDW) in pure Cr in both the low temperature longitudinally polarized phase (T < 122K) and in the higher temperature transversely polarized phase (122K < T < 312K). In both phases spin wave modes of very high velocity are observed originating from the incommensurate Bragg points. In the transversely polarized SDW phase new additional excitations are observed, centered in reciprocal space at the (1,0,0) commensurate point. These excitations are not affected by a magnetic field. Inelastic scattering in the paramagnetic phase above the Neel point (312K) is observed in a reasonably well localized region of reciprocal space near (1,0,0) indicating that there are spin-spin correlations extending over many bcc unit cells and persisting to temperatures at least as high as 1.7 T/sub N/.

  20. Generating coherent states of entangled spins

    SciTech Connect

    Yu Hongyi; Luo Yu; Yao Wang

    2011-09-15

    A coherent state of many spins contains quantum entanglement, which increases with a decrease in the collective spin value. We present a scheme to engineer this class of pure state based on incoherent spin pumping with a few collective raising or lowering operators. In a pumping scenario aimed for maximum entanglement, the steady state of N-pumped spin qubits realizes the ideal resource for the 1{yields}(N/2) quantum telecloning. We show how the scheme can be implemented in a realistic system of atomic spin qubits in an optical lattice. Error analysis shows that high-fidelity state engineering is possible for N{approx}O(100) spins in the presence of decoherence. The scheme can also prepare a resource state for the secret sharing protocol and for the construction of the large-scale Affleck-Kennedy-Lieb-Tasaki state.

  1. Engineering arbitrary pure and mixed quantum states

    SciTech Connect

    Pechen, Alexander

    2011-10-15

    Controlled manipulation by atomic- and molecular-scale quantum systems has attracted a lot of research attention in recent years. A fundamental problem is to provide deterministic methods for controlled engineering of arbitrary quantum states. This work proposes a deterministic method for engineering arbitrary pure and mixed states of a wide class of quantum systems. The method exploits a special combination of incoherent and coherent controls (incoherent and coherent radiation) and has two properties which are specifically important for manipulating by quantum systems: it realizes the strongest possible degree of their state control, complete density matrix controllability, meaning the ability to steer arbitrary pure and mixed initial states into any desired pure or mixed final state, and it is all-to-one, such that each particular control transfers all initial system states into one target state.

  2. New Formulation of Statistical Mechanics Using Thermal Pure Quantum States

    NASA Astrophysics Data System (ADS)

    Sugiura, Sho; Shimizu, Akira

    2014-03-01

    We formulate statistical mechanics based on a pure quantum state, which we call a "thermal pure quantum (TPQ) state". A single TPQ state gives not only equilibrium values of mechanical variables, such as magnetization and correlation functions, but also those of genuine thermodynamic variables and thermodynamic functions, such as entropy and free energy. Among many possible TPQ states, we discuss the canonical TPQ state, the TPQ state whose temperature is specified. In the TPQ formulation of statistical mechanics, thermal fluctuations are completely included in quantum-mechanical fluctuations. As a consequence, TPQ states have much larger quantum entanglement than the equilibrium density operators of the ensemble formulation. We also show that the TPQ formulation is very useful in practical computations, by applying the formulation to a frustrated two-dimensional quantum spin system.

  3. Optimally Squeezed Spin States

    NASA Astrophysics Data System (ADS)

    Rojo, Alberto

    2004-03-01

    We consider optimally spin-squeezed states that maximize the sensitivity of the Ramsey spectroscopy, and for which the signal to noise ratio scales as the number of particles N. Using the variational principle we prove that these states are eigensolutions of the Hamiltonian H(λ)=λ S_z^2-S_x, and that, for large N, the states become equivalent to the quadrature squeezed states of the harmonic oscillator. We present numerical results that illustrate the validity of the equivalence. We also present results of spin squeezing via atom-field interactions within the context of the Tavis-Cummings model. An ensemble of N two-level atoms interacts with a quantized cavity field. For all the atoms initially in their ground states, it is shown that spin squeezing of both the atoms and the field can be achieved provided the initial state of the cavity field has coherence between number states differing by 2. Most of the discussion is restricted to the case of a cavity field initially in a coherent state, but initial squeezed states for the field are also discussed. An analytic solution is found that is valid in the limit that the number of atoms is much greater than unity. References: A. G. Rojo, Phys. Rev A, 68, 013807 (2003); Claudiu Genes, P. R. Berman, and A. G. Rojo Phys. Rev. A 68, 043809 (2003).

  4. Graphical calculus for Gaussian pure states

    SciTech Connect

    Menicucci, Nicolas C.; Flammia, Steven T.; Loock, Peter van

    2011-04-15

    We provide a unified graphical calculus for all Gaussian pure states, including graph transformation rules for all local and semilocal Gaussian unitary operations, as well as local quadrature measurements. We then use this graphical calculus to analyze continuous-variable (CV) cluster states, the essential resource for one-way quantum computing with CV systems. Current graphical approaches to CV cluster states are only valid in the unphysical limit of infinite squeezing, and the associated graph transformation rules only apply when the initial and final states are of this form. Our formalism applies to all Gaussian pure states and subsumes these rules in a natural way. In addition, the term 'CV graph state' currently has several inequivalent definitions in use. Using this formalism we provide a single unifying definition that encompasses all of them. We provide many examples of how the formalism may be used in the context of CV cluster states: defining the 'closest' CV cluster state to a given Gaussian pure state and quantifying the error in the approximation due to finite squeezing; analyzing the optimality of certain methods of generating CV cluster states; drawing connections between this graphical formalism and bosonic Hamiltonians with Gaussian ground states, including those useful for CV one-way quantum computing; and deriving a graphical measure of bipartite entanglement for certain classes of CV cluster states. We mention other possible applications of this formalism and conclude with a brief note on fault tolerance in CV one-way quantum computing.

  5. Ground State Spin Logic

    NASA Astrophysics Data System (ADS)

    Whitfield, James; Faccin, Mauro; Biamonte, Jacob

    2013-03-01

    Designing and optimizing cost functions and energy landscapes is a problem encountered in many fields of science and engineering. These landscapes and cost functions can be embedded and annealed in experimentally controllable spin Hamiltonians. Using an approach based on group theory and symmetries, we examine the embedding of Boolean logic gates into the ground-state subspace of such spin systems. We describe parameterized families of diagonal Hamiltonians and symmetry operations which preserve the ground-state subspace encoding the truth tables of Boolean formulas. The ground-state embeddings of adder circuits are used to illustrate how gates are combined and simplified using symmetry. Our work is relevant for experimental demonstrations of ground-state embeddings found in both classical optimization as well as adiabatic quantum optimization.

  6. Obtaining pure steady states in nonequilibrium quantum systems with strong dissipative couplings

    NASA Astrophysics Data System (ADS)

    Popkov, Vladislav; Presilla, Carlo

    2016-02-01

    Dissipative preparation of a pure steady state usually involves a commutative action of a coherent and a dissipative dynamics on the target state. Namely, the target pure state is an eigenstate of both the coherent and dissipative parts of the dynamics. We show that working in the Zeno regime, i.e., for infinitely large dissipative coupling, one can generate a pure state by a noncommutative action, in the above sense, of the coherent and dissipative dynamics. A corresponding Zeno regime pureness criterion is derived. We illustrate the approach, looking at both its theoretical and applicative aspects, in the example case of an open X X Z spin-1 /2 chain, driven out of equilibrium by boundary reservoirs targeting different spin orientations. Using our criterion, we find two families of pure nonequilibrium steady states, in the Zeno regime, and calculate the dissipative strengths effectively needed to generate steady states which are almost indistinguishable from the target pure states.

  7. Non-Hermitian Hamiltonians and stability of pure states

    NASA Astrophysics Data System (ADS)

    Zloshchastiev, Konstantin G.

    2015-11-01

    We demonstrate that quantum fluctuations can cause, under certain conditions, the dynamical instability of pure states that can result in their evolution into mixed states. It is shown that the degree and type of such an instability are controlled by the environment-induced anti-Hermitian terms in Hamiltonians. Using the quantum-statistical approach for non-Hermitian Hamiltonians and related non-linear master equation, we derive the equations that are necessary to study the stability properties of any model described by a non-Hermitian Hamiltonian. It turns out that the instability of pure states is not preassigned in the evolution equation but arises as the emergent phenomenon in its solutions. In order to illustrate the general formalism and different types of instability that may occur, we perform the local stability analysis of some exactly solvable two-state models, which are being used in the theories of open quantum-optical and spin systems.

  8. Local Unitary Invariant Spin-Squeezing in Multiqubit States

    NASA Astrophysics Data System (ADS)

    Divyamani, B. G.; Sudha; Usha Devi, A. R.

    2016-05-01

    We investiage Local Unitary Invariant Spin Squeezing (LUISS) in symmetric and non-symmetric multiqubit states. On developing an operational procedure to evaluate Local Unitary Invariant Spin Squeezing parameters, we explicitly evaluate these parameters for pure as well as mixed non-symmetric multiqubit states. We show that the existence of local unitary invariant version of Kitegawa-Ueda spin squeezing may not witness pairwise entanglement whereas the local unitary invariant analogue of Wineland spin squeezing necessarily implies pairwise entanglement.

  9. Entanglement entropy of multipartite pure states

    SciTech Connect

    Bravyi, Sergei

    2003-01-01

    Consider a system consisting of n d-dimensional quantum particles and an arbitrary pure state vertical bar {psi}> of the whole system. Suppose we simultaneously perform complete von Neumann measurements on each particle. The Shannon entropy of the outcomes' joint probability distribution is a functional of the state vertical bar {psi}> and of n measurements chosen for each particle. Denote S[{psi}] the minimum of this entropy over all choices of the measurements. We show that S[{psi}] coincides with the entropy of entanglement for bipartite states. We compute S[{psi}] for some special multipartite states: the hexacode state vertical bar H> (n=6, d=2) and the determinant states vertical bar Det{sub n}> (d=n). The computation yields S[H]=4 log 2 and S[Det{sub n}]=log(n{exclamation_point}). Counterparts of the determinant state defined for d

  10. Are all maximally entangled states pure?

    NASA Astrophysics Data System (ADS)

    Cavalcanti, D.; Brandão, F. G. S. L.; Terra Cunha, M. O.

    2005-10-01

    We study if all maximally entangled states are pure through several entanglement monotones. In the bipartite case, we find that the same conditions which lead to the uniqueness of the entropy of entanglement as a measure of entanglement exclude the existence of maximally mixed entangled states. In the multipartite scenario, our conclusions allow us to generalize the idea of the monogamy of entanglement: we establish the polygamy of entanglement, expressing that if a general state is maximally entangled with respect to some kind of multipartite entanglement, then it is necessarily factorized of any other system.

  11. Are all maximally entangled states pure?

    SciTech Connect

    Cavalcanti, D.; Brandao, F.G.S.L.; Terra Cunha, M.O.

    2005-10-15

    We study if all maximally entangled states are pure through several entanglement monotones. In the bipartite case, we find that the same conditions which lead to the uniqueness of the entropy of entanglement as a measure of entanglement exclude the existence of maximally mixed entangled states. In the multipartite scenario, our conclusions allow us to generalize the idea of the monogamy of entanglement: we establish the polygamy of entanglement, expressing that if a general state is maximally entangled with respect to some kind of multipartite entanglement, then it is necessarily factorized of any other system.

  12. Effective pure states for bulk quantum computation

    SciTech Connect

    Knill, E.; Chuang, I.; Laflamme, R.

    1997-11-01

    In bulk quantum computation one can manipulate a large number of indistinguishable quantum computers by parallel unitary operations and measure expectation values of certain observables with limited sensitivity. The initial state of each computer in the ensemble is known but not pure. Methods for obtaining effective pure input states by a series of manipulations have been described by Gershenfeld and Chuang (logical labeling) and Corey et al. (spatial averaging) for the case of quantum computation with nuclear magnetic resonance. We give a different technique called temporal averaging. This method is based on classical randomization, requires no ancilla qubits and can be implemented in nuclear magnetic resonance without using gradient fields. We introduce several temporal averaging algorithms suitable for both high temperature and low temperature bulk quantum computing and analyze the signal to noise behavior of each.

  13. Effective pure states for bulk quantum computation

    SciTech Connect

    Knill, E.; Chuang, I.; Laflamme, R.

    1998-05-01

    In bulk quantum computation one can manipulate a large number of indistinguishable quantum computers by parallel unitary operations and measure expectation values of certain observables with limited sensitivity. The initial state of each computer in the ensemble is known but not pure. Methods for obtaining effective pure input states by a series of manipulations have been described by Gershenfeld and Chuang (logical labeling) [Science {bold 275}, 350 (1997)] and Cory {ital et al.} (spatial averaging) [Proc. Natl. Acad. Sci. USA {bold 94}, 1634 (1997)] for the case of quantum computation with nuclear magnetic resonance. We give a different technique called temporal averaging. This method is based on classical randomization, requires no ancilla quantum bits, and can be implemented in nuclear magnetic resonance without using gradient fields. We introduce several temporal averaging algorithms suitable for both high-temperature and low-temperature bulk quantum computing and analyze the signal-to-noise behavior of each. Most of these algorithms require only a constant multiple of the number of experiments needed by the other methods for creating effective pure states. {copyright} {ital 1998} {ital The American Physical Society}

  14. Entanglement purification protocol for a mixture of a pure entangled state and a pure product state

    SciTech Connect

    Czechlewski, Mikolaj; Wojcik, Antoni; Grudka, Andrzej; Ishizaka, Satoshi

    2009-07-15

    We present an entanglement purification protocol for a mixture of a pure entangled state and a pure product state, which are orthogonal to each other. The protocol is a combination of bisection method and one-way hashing protocol. We give recursive formula for the rate of the protocol for different states, i.e., the number of maximally entangled two-qubit pairs obtained with the protocol per a single copy of the initial state. We also calculate numerically the rate for some states.

  15. Parametric separation of symmetric pure quantum states

    NASA Astrophysics Data System (ADS)

    Solís-Prosser, M. A.; Delgado, A.; Jiménez, O.; Neves, L.

    2016-01-01

    Quantum state separation is a probabilistic map that transforms a given set of pure states into another set of more distinguishable ones. Here we investigate such a map acting onto uniparametric families of symmetric linearly dependent or independent quantum states. We obtained analytical solutions for the success probability of the maps—which is shown to be optimal—as well as explicit constructions in terms of positive operator valued measures. Our results can be used for state discrimination strategies interpolating continuously between minimum-error and unambiguous (or maximum-confidence) discrimination, which, in turn, have many applications in quantum information protocols. As an example, we show that quantum teleportation through a nonmaximally entangled quantum channel can be accomplished with higher probability than the one provided by unambiguous (or maximum-confidence) discrimination and with higher fidelity than the one achievable by minimum-error discrimination. Finally, an optical network is proposed for implementing parametric state separation.

  16. Proposal for direct measurement of a pure spin current by a polarized light beam.

    PubMed

    Wang, Jing; Zhu, Bang-Fen; Liu, Ren-Bao

    2008-02-29

    The photon helicity may be mapped to a spin-1/2, whereby we put forward an intrinsic interaction between a polarized light beam as a "photon spin current" and a pure spin current in a semiconductor, which arises from the spin-orbit coupling in valence bands as a pure relativity effect without involving the Rashba or the Dresselhaus effect due to inversion asymmetries. The interaction leads to linear and circular optical birefringence, which are similar to the Voigt effect and the Faraday rotation in magneto-optics but nevertheless involve no net magnetization. The birefringence effects provide a direct, nondemolition measurement of pure spin currents. PMID:18352646

  17. Fock expansion of multimode pure Gaussian states

    SciTech Connect

    Cariolaro, Gianfranco; Pierobon, Gianfranco

    2015-12-15

    The Fock expansion of multimode pure Gaussian states is derived starting from their representation as displaced and squeezed multimode vacuum states. The approach is new and appears to be simpler and more general than previous ones starting from the phase-space representation given by the characteristic or Wigner function. Fock expansion is performed in terms of easily evaluable two-variable Hermite–Kampé de Fériet polynomials. A relatively simple and compact expression for the joint statistical distribution of the photon numbers in the different modes is obtained. In particular, this result enables one to give a simple characterization of separable and entangled states, as shown for two-mode and three-mode Gaussian states.

  18. Generation and coherent control of pure spin currents via terahertz pulses

    SciTech Connect

    Schüler, Michael Berakdar, Jamal

    2014-04-21

    We inspect the time and spin-dependent, inelastic tunneling in engineered semiconductor-based double quantum well driven by time-structured terahertz pulses. An essential ingredient is an embedded spin-active structure with vibrational modes that scatter the pulse driven carriers. Due to the different time scales of the charge and spin dynamics, the spin-dependent electron-vibron coupling may result in pure net spin current (with negligible charge current). Heating the vibrational site may affect the resulting spin current. Furthermore, by controlling the charge dynamics, the spin dynamics and the generated spin current can be manipulated and switched on and off coherently.

  19. Interaction between spin-wave excitations and pure spin currents in magnetic structures

    NASA Astrophysics Data System (ADS)

    Azevedo, Antonio

    2012-02-01

    The generation of pure spin current (PSC) in magnetic structures has attracted much attention not only for its fundamental importance in spintronics, but also because it opens up potential applications. One of the most exciting aspects of this area is the interplay between spin-waves (SW) and PSC. Here we report experimental results in which the PSC, generated by both spin pumping (SPE) [1] and spin Seebeck (SSE) [2] effects, can exert a spin-transfer torque sufficient to compensate the SW relaxation in yttrium iron garnet (YIG)/non-magnetic structures. By measuring the propagation of SW packets in single-crystal YIG films we were able to observe the amplification of volume and magnetostatic modes (MSW) by both SSE and SHE [3,4]. The excitation and detection of the SW packets is carried out by using a MSW delay line device. In both cases the amplification is attributed to the spin-transfer torque due to PSC generated by SSE as well as SHE. It will also be presented new results in which PSC are simultaneously excited by SSE and SPE effects in YIG films. While the spin current generated by SPE is obtained by exciting the ferromagnetic resonance (FMR) of the YIG film, the spin current due to SSE is created by applying a temperature gradient along the film plane. The effect of the superposition of both spin currents is characterized by measuring the spin Hall voltage (VH) along thin strips of Pt deposited on top of the YIG films. Whereas VH corresponding to the uniform FMR is amplified due the SSE the voltages corresponding to the other magnetostatic spin-wave modes are attenuated [5]. [4pt] [1] Y. Tserkovnyak, et al., Rev. Mod. Phys. 77, 1375 (2005).[0pt] [2] K. Uchida, et al., Nature 455, 778 (2008).[0pt] [3] E. Padr'on-Hern'andez, A. Azevedo, and S. M. Rezende, Phys. Rev. Letts., 107, 197203 (2011).[0pt] [4] E. Padr'on-Hern'andez, A. Azevedo, and S. M. Rezende, Appl. Phys. Letts., 99 (2011) in press.[0pt] [5] G.L. da Silva, L.H. Vilela-Leão, S. M. Rezende and A

  20. Voltage-controllable generator of pure spin current: A three-terminal model

    SciTech Connect

    Ma, Zheng; Wu, Reng-Lai; Yu, Ya-Bin Wang, Miao

    2014-07-28

    Three-terminal devices have been frequently proposed to generate the pure spin current. However, the controllability and stability of pure spin current still needs to be improved. In this paper, a three-terminal device, composed of a ferromagnetic metallic lead and two nonmagnetic semiconductor leads coupled with a quantum dot, is employed to study the properties of electron spin transport. The results show that when the external voltage on one of nonmagnetic semiconductor leads is adjusted to a proper range, a pure spin current plateau or a fully spin-polarized current plateau appears in another nonmagnetic semiconductor lead. In a wide range of external voltage, the pure spin current or the spin-polarized current is kept unchanged. Since the change of temperature may considerably influence the spin-polarization of current and is inevitable actually, we studied the corresponding compensation to keep the pure spin current unchanged. Furthermore, the effect of device parameters on the pure spin current is also investigated.

  1. Visualizing spin states using the spin coherent state representation

    NASA Astrophysics Data System (ADS)

    Lee Loh, Yen; Kim, Monica

    2015-01-01

    Orbital angular momentum eigenfunctions are readily understood in terms of spherical harmonics. However, the quantum mechanical phenomenon of spin is often said to be mysterious and hard to visualize, with no classical analog. Many textbooks give a heuristic and somewhat unsatisfying picture of a precessing spin vector. Here, we show that the spin-coherent-state representation is a striking, elegant, and mathematically meaningful tool for visualizing spin states. We also demonstrate that cartographic projections such as the Hammer projection are useful for visualizing functions defined on spherical surfaces.

  2. Hologram of a pure state black hole

    NASA Astrophysics Data System (ADS)

    Roy, Shubho R.; Sarkar, Debajyoti

    2015-12-01

    In this paper, we extend the Hamilton-Kabat-Lifschytz-Lowe (HKLL) holographic smearing function method to reconstruct (quasi)local anti-de Sitter bulk scalar observables in the background of a large anti-de Sitter black hole formed by null shell collapse (a "pure state" black hole), from the dual conformal field theory which is undergoing a sudden quench. In particular, we probe the near horizon and subhorizon bulk locality. First, we construct local bulk operators from the conformal field theory in the leading semiclassical limit, N →∞ . Then, we look at effects due to the finiteness of N , where we propose a suitable coarse-graining prescription involving early and late time cutoffs to define semiclassical bulk observables which are approximately local, their departure from locality being nonperturbatively small in N . Our results have important implications on the black hole information problem.

  3. Manipulation of pure spin current in ferromagnetic metals independent of magnetization

    NASA Astrophysics Data System (ADS)

    Tian, Dai; Li, Yufan; Qu, D.; Huang, S. Y.; Jin, Xiaofeng; Chien, C. L.

    2016-07-01

    Upon the injection of a pure spin current, a ferromagnet, similar to a nonmagnetic metal, also exhibits inverse spin Hall effect (ISHE). We show in Co/Cu/YIG, where the thin Cu layer allows transmission of spin current from YIG into Co but decouples the two ferromagnets, that the interaction between ISHE and ferromagnetic ordering in Co can be unambiguously investigated. By switching on and off the pure spin current contribution, we demonstrate that the ISHE in Co is independent of the direction of the Co magnetization, which clearly suggests that the ISHE in Co is dominated not by the extrinsic impurity scatterings, but from the intrinsic origin.

  4. Nonadiabatic pure spin pumping in zigzag graphene nanoribbons with proximity induced ferromagnetism

    NASA Astrophysics Data System (ADS)

    Cheraghchi, Hosein

    2016-01-01

    By combining Floquet theory with Green's function formalism, we present non-adiabatic quantum spin and charge pumping through a zigzag ferromagnetic graphene nanoribbon including a double-barriers structure driven weakly by two local ac gate voltages operating with a phase-lag. Over a wide range of Fermi energies, interesting quantum pumping such as (i) pure spin pumping with zero net charge pumping, (ii) pure charge pumping and (iii) fully spin polarized pumping can be achieved by tuning and manipulating driving frequency in the non-adiabatic regime. Spin polarized pumping which is measurable using the current technology depends on the competition between the energy level spacing and the driving frequency.

  5. Optimal single quantum dot heat-to-pure-spin-current converters

    NASA Astrophysics Data System (ADS)

    Buddhiraju, Siddharth; Muralidharan, Bhaskaran

    2015-12-01

    We delve into the conditions under which a quantum dot thermoelectric setup may be tuned to realize an optimal heat-to-pure-spin-current converter. It is well known that a heat-to-pure-spin-current converter may be realized using a non-interacting quantum dot with a spin-split energy spectrum under particle hole symmetry conditions. However, with the inclusion of Coulomb interaction U, ubiquitous in typical quantum dot systems, the relevant transport physics is expected to be altered. In this work, we provide a detailed picture of thermoelectric pure spin currents at various Coulomb interaction parameters U and describe the conditions necessary for an exact cancelation of charge transport between energy levels ɛ and their Coulomb-charged partner levels ɛ + U, so as to yield the largest terminal pure spin currents. A non-trivial aspect pointed out here is that at sufficiently large values of U (≥ U0), pure spin currents tend to optimize at points other than where the particle-hole symmetry occurs. It is also ascertained that a global maximum of pure spin current is generated at a typical value of the interaction parameter U. These optimum conditions may be easily realized using a typical gated quantum dot thermoelectric transport setup.

  6. Entanglement bound for multipartite pure states based on local measurements

    SciTech Connect

    Jiang Lizhen; Chen Xiaoyu; Ye Tianyu

    2011-10-15

    An entanglement bound based on local measurements is introduced for multipartite pure states. It is the upper bound of the geometric measure and the relative entropy of entanglement. It is the lower bound of the minimal-measurement entropy. For pure bipartite states, the bound is equal to the entanglement entropy. The bound is applied to pure tripartite qubit states and the exact tripartite relative entropy of entanglement is obtained for a wide class of states.

  7. Thermally Driven Pure Spin and Valley Currents via the Anomalous Nernst Effect in Monolayer Group-VI Dichalcogenides.

    PubMed

    Yu, Xiao-Qin; Zhu, Zhen-Gang; Su, Gang; Jauho, A-P

    2015-12-11

    The spin and valley-dependent anomalous Nernst effects are analyzed for monolayer MoS_{2} and other group-VI dichalcogenides. We find that pure spin and valley currents can be generated perpendicular to the applied thermal gradient in the plane of these two-dimensional materials. This effect provides a versatile platform for applications of spin caloritronics. A spin current purity factor is introduced to quantify this effect. When time reversal symmetry is violated, e.g., two-dimensional materials on an insulating magnetic substrate, a dip-peak feature appears for the total Nernst coefficient. For the dip state it is found that carriers with only one spin and from one valley are driven by the temperature gradient. PMID:26705646

  8. Pure collective precession motion of a high-spin torus isomer

    NASA Astrophysics Data System (ADS)

    Ichikawa, T.; Matsuyanagi, K.; Maruhn, J. A.; Itagaki, N.

    2014-01-01

    We investigate the precession motion of the exotic torus configuration in high-spin excited states of 40Ca. For this aim, we use the three-dimensional time-dependent Hartree-Fock (TDHF) method. Although the high-spin torus isomer is a unique quantum object characterized by the alignment of angular momenta of independent single-particle motions, we find that the obtained moment of inertia for rotations about an axis perpendicular to the symmetry axis is close to the rigid-body value. We also analyze the microscopic structure of the precession motion using the random-phase approximation (RPA) method for high-spin states. In the RPA calculation, the precession motion of the torus isomer is generated by coherent superposition of many one-particle-one-hole excitations across the sloping Fermi surface that strongly violates the time-reversal symmetry. By comparing results of the TDHF and the RPA calculations, we find that the precession motion obtained by the TDHF calculation is a pure collective motion well decoupled from other collective modes.

  9. Direct observation of dynamic modes excited in a magnetic insulator by pure spin current.

    PubMed

    Demidov, V E; Evelt, M; Bessonov, V; Demokritov, S O; Prieto, J L; Muñoz, M; Ben Youssef, J; Naletov, V V; de Loubens, G; Klein, O; Collet, M; Bortolotti, P; Cros, V; Anane, A

    2016-01-01

    Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533

  10. Direct observation of dynamic modes excited in a magnetic insulator by pure spin current

    PubMed Central

    Demidov, V. E.; Evelt, M.; Bessonov, V.; Demokritov, S. O.; Prieto, J. L.; Muñoz, M.; Ben Youssef, J.; Naletov, V. V.; de Loubens, G.; Klein, O.; Collet, M.; Bortolotti, P.; Cros, V.; Anane, A.

    2016-01-01

    Excitation of magnetization dynamics by pure spin currents has been recently recognized as an enabling mechanism for spintronics and magnonics, which allows implementation of spin-torque devices based on low-damping insulating magnetic materials. Here we report the first spatially-resolved study of the dynamic modes excited by pure spin current in nanometer-thick microscopic insulating Yttrium Iron Garnet disks. We show that these modes exhibit nonlinear self-broadening preventing the formation of the self-localized magnetic bullet, which plays a crucial role in the stabilization of the single-mode magnetization oscillations in all-metallic systems. This peculiarity associated with the efficient nonlinear mode coupling in low-damping materials can be among the main factors governing the interaction of pure spin currents with the dynamic magnetization in high-quality magnetic insulators. PMID:27608533

  11. Spin Charge Separation in the Quantum Spin Hall State

    SciTech Connect

    Qi, Xiao-Liang; Zhang, Shou-Cheng; /Stanford U., Phys. Dept.

    2010-03-19

    The quantum spin Hall state is a topologically non-trivial insulator state protected by the time reversal symmetry. We show that such a state always leads to spin-charge separation in the presence of a {pi} flux. Our result is generally valid for any interacting system. We present a proposal to experimentally observe the phenomenon of spin-charge separation in the recently discovered quantum spin Hall system.

  12. Conversion of pure spin current to charge current in amorphous bismuth

    SciTech Connect

    Emoto, H.; Ando, Y.; Shinjo, T.; Shiraishi, M.; Shikoh, E.; Fuseya, Y.

    2014-05-07

    Spin Hall angle and spin diffusion length in amorphous bismuth (Bi) are investigated by using conversion of a pure spin current to a charge current in a spin pumping technique. In Bi/Ni{sub 80}Fe{sub 20}/Si(100) sample, a clear direct current (DC) electromotive force due to the inverse spin Hall effect of the Bi layer is observed at room temperature under a ferromagnetic resonance condition of the Ni{sub 80}Fe{sub 20} layer. From the Bi thickness dependence of the DC electromotive force, the spin Hall angle and the spin diffusion length of the amorphous Bi film are estimated to be 0.02 and 8 nm, respectively.

  13. Ground-state spin logic

    NASA Astrophysics Data System (ADS)

    Whitfield, J. D.; Faccin, M.; Biamonte, J. D.

    2012-09-01

    Designing and optimizing cost functions and energy landscapes is a problem encountered in many fields of science and engineering. These landscapes and cost functions can be embedded and annealed in experimentally controllable spin Hamiltonians. Using an approach based on group theory and symmetries, we examine the embedding of Boolean logic gates into the ground-state subspace of such spin systems. We describe parameterized families of diagonal Hamiltonians and symmetry operations which preserve the ground-state subspace encoding the truth tables of Boolean formulas. The ground-state embeddings of adder circuits are used to illustrate how gates are combined and simplified using symmetry. Our work is relevant for experimental demonstrations of ground-state embeddings found in both classical optimization as well as adiabatic quantum optimization.

  14. Direct Detection of Pure ac Spin Current by X-Ray Pump-Probe Measurements.

    PubMed

    Li, J; Shelford, L R; Shafer, P; Tan, A; Deng, J X; Keatley, P S; Hwang, C; Arenholz, E; van der Laan, G; Hicken, R J; Qiu, Z Q

    2016-08-12

    Despite recent progress in spin-current research, the detection of spin current has mostly remained indirect. By synchronizing a microwave waveform with synchrotron x-ray pulses, we use the ferromagnetic resonance of the Py (Ni_{81}Fe_{19}) layer in a Py/Cu/Cu_{75}Mn_{25}/Cu/Co multilayer to pump a pure ac spin current into the Cu_{75}Mn_{25} and Co layers, and then directly probe the spin current within the Cu_{75}Mn_{25} layer and the spin dynamics of the Co layer by x-ray magnetic circular dichroism. This element-resolved pump-probe measurement unambiguously identifies the ac spin current in the Cu_{75}Mn_{25} layer. PMID:27563981

  15. Direct Detection of Pure ac Spin Current by X-Ray Pump-Probe Measurements

    NASA Astrophysics Data System (ADS)

    Li, J.; Shelford, L. R.; Shafer, P.; Tan, A.; Deng, J. X.; Keatley, P. S.; Hwang, C.; Arenholz, E.; van der Laan, G.; Hicken, R. J.; Qiu, Z. Q.

    2016-08-01

    Despite recent progress in spin-current research, the detection of spin current has mostly remained indirect. By synchronizing a microwave waveform with synchrotron x-ray pulses, we use the ferromagnetic resonance of the Py (Ni81Fe19 ) layer in a Py /Cu /Cu75Mn25/Cu /Co multilayer to pump a pure ac spin current into the Cu75Mn25 and Co layers, and then directly probe the spin current within the Cu75Mn25 layer and the spin dynamics of the Co layer by x-ray magnetic circular dichroism. This element-resolved pump-probe measurement unambiguously identifies the ac spin current in the Cu75Mn25 layer.

  16. Note about a pure spin-connection formulation of general relativity and spin-2 duality in (A)dS

    NASA Astrophysics Data System (ADS)

    Basile, Thomas; Bekaert, Xavier; Boulanger, Nicolas

    2016-06-01

    We investigate the problem of finding a pure spin-connection formulation of general relativity with nonvanishing cosmological constant. We first revisit the problem at the linearized level and find that the pure spin-connection, quadratic Lagrangian, takes a form reminiscent to Weyl gravity, given by the square of a Weyl-like tensor. Upon Hodge dualization, we show that the dual gauge field in (A )dSD transforms under G L (D ) in the same representation as a massive graviton in the flat spacetime of the same dimension. We give a detailed proof that the physical degrees of freedom indeed correspond to a massless graviton propagating around the (anti-) de Sitter background and finally speculate about a possible nonlinear pure-connection theory dual to general relativity with cosmological constant.

  17. Squeezed spin states: Squeezing the spin uncertainty relations

    NASA Technical Reports Server (NTRS)

    Kitagawa, Masahiro; Ueda, Masahito

    1993-01-01

    The notion of squeezing in spin systems is clarified, and the principle for spin squeezing is shown. Two twisting schemes are proposed as building blocks for spin squeezing and are shown to reduce the standard quantum noise, s/2, of the coherent S-spin state down to the order of S(sup 1/3) and 1/2. Applications to partition noise suppression are briefly discussed.

  18. Pure-state informationally complete and 'really' complete measurements

    SciTech Connect

    Finkelstein, J.

    2004-11-01

    I construct a positive-operator-valued measure (POVM) which has 2d rank-1 elements and which is informationally complete for generic pure states in d dimensions, thus confirming a conjecture made by Flammia, Silberfarb, and Caves (e-print quant-ph/0404137). I show that if a rank-1 POVM is required to be informationally complete for all pure states in d dimensions, it must have at least 3d-2 elements. I also show that, in a POVM which is informationally complete for all pure states in d dimensions, for any vector there must be at least 2d-1 POVM elements which do not annihilate that vector.

  19. Typical pure nonequilibrium steady states and irreversibility for quantum transport.

    PubMed

    Monnai, Takaaki; Yuasa, Kazuya

    2016-07-01

    It is known that each single typical pure state in an energy shell of a large isolated quantum system well represents a thermal equilibrium state of the system. We show that such typicality holds also for nonequilibrium steady states (NESS's). We consider a small quantum system coupled to multiple infinite reservoirs. In the long run, the total system reaches a unique NESS. We identify a large Hilbert space from which pure states of the system are to be sampled randomly and show that the typical pure states well describe the NESS. We also point out that the irreversible relaxation to the unique NESS is important to the typicality of the pure NESS's. PMID:27575115

  20. State diagram of an orthogonal spin transfer spin valve device

    SciTech Connect

    Ye, Li; Wolf, Georg; Pinna, Daniele; Chaves-O'Flynn, Gabriel D.; Kent, Andrew D.

    2015-05-21

    We present the switching characteristics of a spin-transfer device that incorporates a perpendicularly magnetized spin-polarizing layer with an in-plane magnetized free and fixed magnetic layer, known as an orthogonal spin transfer spin valve device. This device shows clear switching between parallel (P) and antiparallel (AP) resistance states and the reverse transition (AP → P) for both current polarities. Further, hysteretic transitions are shown to occur into a state with a resistance intermediate between that of the P and AP states, again for both current polarities. These unusual spin-transfer switching characteristics can be explained within a simple macrospin model that incorporates thermal fluctuations and considers a spin-polarized current that is tilted with respect to the free layer's plane, due to the presence of the spin-transfer torque from the polarizing layer.

  1. Single biphoton ququarts as either pure or mixed states

    SciTech Connect

    Fedorov, M. V.; Volkov, P. A.; Mikhailova, J. M.

    2011-09-15

    We analyze features of mixed biphoton polarization states, which arise from pure states of polarization-frequency biphoton ququarts after averaging over frequencies of photons. For mixed states, we find their concurrence C, Schmidt parameter K, degree of polarization P, as well as the von Neumann mutual information I. In some simple cases, we also find the relative entropy S{sub rel} and the degree of classical correlations C{sub cl}. In mixed states, the Schmidt parameter does not characterize the degree of entanglement anymore, as it does in pure states. Nevertheless, the Schmidt parameter remains useful even in the case of mixed states because it remains directly related to the degree of polarization. We compare results occurring in the cases of full pure polarization-frequency states of ququarts and mixed states (averaged over frequencies). Differences between these results can be seen in experiments with and without frequency filters in front of a detector.

  2. Information balance in quantum teleportation with an arbitrary pure state

    SciTech Connect

    Li Li; Chen Zengbing

    2005-07-15

    We study a general teleportation scheme with an arbitrary two-party pure state and derive a tight bound of the teleportation fidelity with a predesigned estimation of the unknown state to be teleported. This bound shows a piecewise balance between information gain and state disturbance. We also explain possible physical significance of the balance.

  3. Detection of pure inverse spin-Hall effect induced by spin pumping at various excitation

    NASA Astrophysics Data System (ADS)

    Inoue, H. Y.; Harii, K.; Ando, K.; Sasage, K.; Saitoh, E.

    2007-10-01

    Electric-field generation due to the inverse spin-Hall effect (ISHE) driven by spin pumping was detected and separated experimentally from the extrinsic magnetogalvanic effects in a Ni81Fe19/Pt film. By applying a sample-cavity configuration in which the extrinsic effects are suppressed, the spin pumping using ferromagnetic resonance gives rise to a symmetric spectral shape in the electromotive force spectrum, indicating that the motive force is due entirely to ISHE. This method allows the quantitative analysis of the ISHE and the spin-pumping effect. The microwave-power dependence of the ISHE amplitude is consistent with the prediction of a direct current-spin-pumping scenario.

  4. All-spin nanomagnetic state elements

    NASA Astrophysics Data System (ADS)

    Manipatruni, Sasikanth; Nikonov, Dmitri E.; Young, Ian A.

    2013-08-01

    We propose an all-spin state element using spin currents and nanomagnets to enable all-spin state machines for digital computing. We demonstrate via numerical simulations the operation of the state element, a critical building block for synchronous, sequential logic computation. The numerical models encompass Landau-Lifshitz-Gilbert nanomagnet dynamics with stochastic models and vector spin-transport in metallic magnetic and non-magnetic channels. Combined with all-spin combinatorial logic, the state elements can enable synchronous and asynchronous computing elements.

  5. Fisher-Symmetric Informationally Complete Measurements for Pure States.

    PubMed

    Li, Nan; Ferrie, Christopher; Gross, Jonathan A; Kalev, Amir; Caves, Carlton M

    2016-05-01

    We introduce a new kind of quantum measurement that is defined to be symmetric in the sense of uniform Fisher information across a set of parameters that uniquely represent pure quantum states in the neighborhood of a fiducial pure state. The measurement is locally informationally complete-i.e., it uniquely determines these parameters, as opposed to distinguishing two arbitrary quantum states-and it is maximal in the sense of a multiparameter quantum Cramér-Rao bound. For a d-dimensional quantum system, requiring only local informational completeness allows us to reduce the number of outcomes of the measurement from a minimum close to but below 4d-3, for the usual notion of global pure-state informational completeness, to 2d-1. PMID:27203310

  6. Entanglement convertibility for infinite-dimensional pure bipartite states

    SciTech Connect

    Owari, Masaki; Matsumoto, Keiji; Murao, Mio

    2004-11-01

    It is shown that the order property of pure bipartite states under stochastic local operations and classical communications (SLOCC) changes radically when dimensionality shifts from finite to infinite. In contrast to finite-dimensional systems where there is no pure incomparable state, the existence of infinitely many mutually SLOCC incomparable states is shown for infinite-dimensional systems even under the bounded energy and finite information exchange condition. These results show that the effect of the infinite dimensionality of Hilbert space, the 'infinite workspace' property, remains even in physically relevant infinite-dimensional systems.

  7. Gaussian-optimized preparation of non-Gaussian pure states

    NASA Astrophysics Data System (ADS)

    Menzies, David; Filip, Radim

    2009-01-01

    Non-Gaussian states are highly sought-after resources in continuous-variable quantum optical information processing protocols. We outline a method for the optimized preparation of any pure non-Gaussian state to a given desired accuracy. Our proposal arises from two connected concepts. First, we define the operational cost of a desired state as the largest Fock state required for its approximate preparation. Second, we suggest that this non-Gaussian operational cost can be reduced by judicial application of optimized Gaussian operations. In particular, we identify a minimal core non-Gaussian state for any target pure state, which is related to the core state by Gaussian operations alone. We demonstrate this method for Schrödinger cat states.

  8. Nonlocality in pure and mixed n-qubit X states

    NASA Astrophysics Data System (ADS)

    Batle, J.; Ooi, C. H. Raymond; Farouk, Ahmed; Abdalla, S.

    2016-04-01

    Nonlocality for general multiqubit X states is studied in detail. Pure and mixed states are analyzed as far as their maximum amount of nonlocality is concerned, and analytic results are obtained for important families of these states. The particular form of nonzero diagonal and antidiagonal matrix elements makes the corresponding study easy enough to obtain exact results. We also provide a numerical recipe to randomly generate an important family of X states endowed with a given degree of mixture.

  9. Fisher-Symmetric Informationally Complete Measurements for Pure States

    NASA Astrophysics Data System (ADS)

    Li, Nan; Ferrie, Christopher; Gross, Jonathan A.; Kalev, Amir; Caves, Carlton M.

    2016-05-01

    We introduce a new kind of quantum measurement that is defined to be symmetric in the sense of uniform Fisher information across a set of parameters that uniquely represent pure quantum states in the neighborhood of a fiducial pure state. The measurement is locally informationally complete—i.e., it uniquely determines these parameters, as opposed to distinguishing two arbitrary quantum states—and it is maximal in the sense of a multiparameter quantum Cramér-Rao bound. For a d -dimensional quantum system, requiring only local informational completeness allows us to reduce the number of outcomes of the measurement from a minimum close to but below 4 d -3 , for the usual notion of global pure-state informational completeness, to 2 d -1 .

  10. Violations of Bell inequalities from random pure states

    NASA Astrophysics Data System (ADS)

    Atkin, Max R.; Zohren, Stefan

    2015-07-01

    We consider the expected violations of Bell inequalities from random pure states. More precisely, we focus on a slightly generalized version of the Collins-Gisin-Linden-Massar-Popescu inequality, which concerns Bell experiments of two parties, two measurement options, and N outcomes, and analyze their expected quantum violations from random pure states for varying N , assuming the conjectured optimal measurement operators. It is seen that for small N the Bell inequality is not violated on average, while for larger N it is. Both ensembles of unstructured as well as structured random pure states are considered. Using techniques from random matrix theory this is obtained analytically for small and large N and numerically for intermediate N . The results show a beautiful interplay of different aspects of random matrix theory, ranging from the Marchenko-Pastur distribution and fixed-trace ensembles to the O (n ) model.

  11. Faithful Transfer Arbitrary Pure States with Mixed Resources

    NASA Astrophysics Data System (ADS)

    Luo, Ming-Xing; Li, Lin; Ma, Song-Ya; Chen, Xiu-Bo; Yang, Yi-Xian

    2013-09-01

    In this paper, we show that some special mixed quantum resource experience the same property of pure entanglement such as Bell state for quantum teleportation. It is shown that one mixed state and three bits of classical communication cost can be used to teleport one unknown qubit compared with two bits via pure resources. The schemes are easily implement with model physical techniques. Moreover, these resources are also optimal and typical for faithfully remotely prepare an arbitrary qubit, two-qubit and three-qubit states with mixed quantum resources. Our schemes are completed as same as those with pure quantum entanglement resources except only 1 bit additional classical communication cost required. The success probability is independent of the form of the mixed resources.

  12. Spin polarization of the split Kondo state.

    PubMed

    von Bergmann, Kirsten; Ternes, Markus; Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

    2015-02-20

    Spin-resolved scanning tunneling microscopy is employed to quantitatively determine the spin polarization of the magnetic field-split Kondo state. Tunneling conductance spectra of a Kondo-screened magnetic atom are evaluated within a simple model taking into account inelastic tunneling due to spin excitations and two Kondo peaks positioned symmetrically around the Fermi energy. We fit the spin state of the Kondo-screened atom with a spin Hamiltonian independent of the Kondo effect and account for Zeeman splitting of the Kondo peak in the magnetic field. We find that the width and the height of the Kondo peaks scales with the Zeeman energy. Our observations are consistent with full spin polarization of the Kondo peaks, i.e., a majority spin peak below the Fermi energy and a minority spin peak above. PMID:25763966

  13. Entropy for quantum pure states and quantum H theorem.

    PubMed

    Han, Xizhi; Wu, Biao

    2015-06-01

    We construct a complete set of Wannier functions that are localized at both given positions and momenta. This allows us to introduce the quantum phase space, onto which a quantum pure state can be mapped unitarily. Using its probability distribution in quantum phase space, we define an entropy for a quantum pure state. We prove an inequality regarding the long-time behavior of our entropy's fluctuation. For a typical initial state, this inequality indicates that our entropy can relax dynamically to a maximized value and stay there most of time with small fluctuations. This result echoes the quantum H theorem proved by von Neumann [Zeitschrift für Physik 57, 30 (1929)]. Our entropy is different from the standard von Neumann entropy, which is always zero for quantum pure states. According to our definition, a system always has bigger entropy than its subsystem even when the system is described by a pure state. As the construction of the Wannier basis can be implemented numerically, the dynamical evolution of our entropy is illustrated with an example. PMID:26172660

  14. Entropy for quantum pure states and quantum H theorem

    NASA Astrophysics Data System (ADS)

    Han, Xizhi; Wu, Biao

    2015-06-01

    We construct a complete set of Wannier functions that are localized at both given positions and momenta. This allows us to introduce the quantum phase space, onto which a quantum pure state can be mapped unitarily. Using its probability distribution in quantum phase space, we define an entropy for a quantum pure state. We prove an inequality regarding the long-time behavior of our entropy's fluctuation. For a typical initial state, this inequality indicates that our entropy can relax dynamically to a maximized value and stay there most of time with small fluctuations. This result echoes the quantum H theorem proved by von Neumann [Zeitschrift für Physik 57, 30 (1929), 10.1007/BF01339852]. Our entropy is different from the standard von Neumann entropy, which is always zero for quantum pure states. According to our definition, a system always has bigger entropy than its subsystem even when the system is described by a pure state. As the construction of the Wannier basis can be implemented numerically, the dynamical evolution of our entropy is illustrated with an example.

  15. Control aspects of quantum computing using pure and mixed states

    PubMed Central

    Schulte-Herbrüggen, Thomas; Marx, Raimund; Fahmy, Amr; Kauffman, Louis; Lomonaco, Samuel; Khaneja, Navin; Glaser, Steffen J.

    2012-01-01

    Steering quantum dynamics such that the target states solve classically hard problems is paramount to quantum simulation and computation. And beyond, quantum control is also essential to pave the way to quantum technologies. Here, important control techniques are reviewed and presented in a unified frame covering quantum computational gate synthesis and spectroscopic state transfer alike. We emphasize that it does not matter whether the quantum states of interest are pure or not. While pure states underly the design of quantum circuits, ensemble mixtures of quantum states can be exploited in a more recent class of algorithms: it is illustrated by characterizing the Jones polynomial in order to distinguish between different (classes of) knots. Further applications include Josephson elements, cavity grids, ion traps and nitrogen vacancy centres in scenarios of closed as well as open quantum systems. PMID:22946034

  16. Groverian entanglement measure of pure quantum states with arbitrary partitions

    SciTech Connect

    Shimoni, Yishai; Biham, Ofer

    2007-02-15

    The Groverian entanglement measure of pure quantum states of n qubits is generalized to the case in which the qubits are divided into any p{<=}n parties. The entanglement between these parties is evaluated numerically using an efficient parametrization. To demonstrate this measure we apply it to symmetric states such as the Greenberg-Horne-Zeiliner state and the W state. Interestingly, this measure is equivalent to an entanglement measure introduced earlier [H. Barnum and N. Linden, J. Phys. A 34, 6787 (2001)], using different considerations.

  17. Probabilistically Perfect Cloning of Two Pure States: Geometric Approach

    NASA Astrophysics Data System (ADS)

    Yerokhin, V.; Shehu, A.; Feldman, E.; Bagan, E.; Bergou, J. A.

    2016-05-01

    We solve the long-standing problem of making n perfect clones from m copies of one of two known pure states with minimum failure probability in the general case where the known states have arbitrary a priori probabilities. The solution emerges from a geometric formulation of the problem. This formulation reveals that cloning converges to state discrimination followed by state preparation as the number of clones goes to infinity. The convergence exhibits a phenomenon analogous to a second-order symmetry-breaking phase transition.

  18. Probabilistically Perfect Cloning of Two Pure States: Geometric Approach.

    PubMed

    Yerokhin, V; Shehu, A; Feldman, E; Bagan, E; Bergou, J A

    2016-05-20

    We solve the long-standing problem of making n perfect clones from m copies of one of two known pure states with minimum failure probability in the general case where the known states have arbitrary a priori probabilities. The solution emerges from a geometric formulation of the problem. This formulation reveals that cloning converges to state discrimination followed by state preparation as the number of clones goes to infinity. The convergence exhibits a phenomenon analogous to a second-order symmetry-breaking phase transition. PMID:27258856

  19. Quantum benchmarks for pure single-mode Gaussian states.

    PubMed

    Chiribella, Giulio; Adesso, Gerardo

    2014-01-10

    Teleportation and storage of continuous variable states of light and atoms are essential building blocks for the realization of large-scale quantum networks. Rigorous validation of these implementations require identifying, and surpassing, benchmarks set by the most effective strategies attainable without the use of quantum resources. Such benchmarks have been established for special families of input states, like coherent states and particular subclasses of squeezed states. Here we solve the longstanding problem of defining quantum benchmarks for general pure Gaussian single-mode states with arbitrary phase, displacement, and squeezing, randomly sampled according to a realistic prior distribution. As a special case, we show that the fidelity benchmark for teleporting squeezed states with totally random phase and squeezing degree is 1/2, equal to the corresponding one for coherent states. We discuss the use of entangled resources to beat the benchmarks in experiments. PMID:24483875

  20. Pure spin-Hall magnetoresistance in Rh/Y3Fe5O12 hybrid.

    PubMed

    Shang, T; Zhan, Q F; Ma, L; Yang, H L; Zuo, Z H; Xie, Y L; Li, H H; Liu, L P; Wang, B M; Wu, Y H; Zhang, S; Li, Run-Wei

    2015-01-01

    We report an investigation of anisotropic magnetoresistance (AMR) and anomalous Hall resistance (AHR) of Rh and Pt thin films sputtered on epitaxial Y(3)Fe(5)O(12) (YIG) ferromagnetic insulator films. For the Pt/YIG hybrid, large spin-Hall magne toresistance (SMR) along with a sizable conventional anisotropic magnetoresistance (CAMR) and a nontrivial temperature dependence of AHR were observed in the temperature range of 5-300 K. In contrast, a reduced SMR with negligible CAMR and AHR was found in Rh/YIG hybrid. Since CAMR and AHR are characteristics for all ferromagnetic metals, our results suggest that the Pt is likely magnetized by YIG due to the magnetic proximity effect (MPE) while Rh remains free of MPE. Thus the Rh/YIG hybrid could be an ideal model system to explore physics and devices associated with pure spin current. PMID:26639108

  1. High-Spin States in 124Ba

    NASA Astrophysics Data System (ADS)

    Al-Khatib, A.; Singh, A. K.; Huebel, H.; Bringel, P.; Buerger, A.; Neusser, A.; Schoenwasser, G.; Hagemann, G. B.; Hansen, C. R.; Herskind, B.; Sletten, G.; Algora, A.; Dombradi, Zs.; Gal, J.; Kalinka, G.; Molnar, J.; Nyako, B. M.; Sohler, D.; Timar, J.; Zolnai, L.; Kmiecik, M.; Maj, A.; Styczen, J.; Zuber, K.; Hauschild, K.; Korichi, A.; Lopez-Martens, A.; Roccaz, J.; Siem, S.; Hannachi, F.; Scheurer, J. N.; Bednarczyk, P.; Byrski, Th.; Curien, D.; Dorvaux, O.; Duchene, G.; Gall, B.; Khalfallah, F.; Piqueras, I.; Robin, J.; Juhasz, K.; Patel, S. B.; Evans, A. O.; Rainovski, G.; Airoldi, A.; Benzoni, G.; Bracco, A.; Camera, F.; Million, B.; Mason, P.; Paleni, A.; Sacchi, R.; Wieland, O.; Petrache, C. M.; Petrache, D.; La Rana, G.; Moro, R.; de Angelis, G.; Fallon, P.; Lee, I.-Y.; Lisle, J. C.; Cederwall, B.; Lagergren, K.; Lieder, R. M.; Podsvirova, E.; Gast, W.; Jaeger, H.; Redon, N.; Goergen, A.

    2005-04-01

    High-spin states in 124Ba were populated using the 64Ni(64Ni,4n)124Ba reaction at beam energies of 255 and 261 MeV. Gamma-ray coincidences were measured using the EUROBALL detector array.The charged-particle detector array DIAMANT provided channel selection. The previously known rotational bands are extended to higher spins. Five new bands are observed, one of them extends up to the spin 40 hbar region.

  2. Push-Pull Optical Pumping of Pure Superposition States

    NASA Astrophysics Data System (ADS)

    Jau, Y.-Y.; Miron, E.; Post, A. B.; Kuzma, N. N.; Happer, W.

    2004-10-01

    A new optical pumping method, “push-pull pumping,” can produce very nearly pure, coherent superposition states between the initial and the final sublevels of the important field-independent 0-0 clock resonance of alkali-metal atoms. The key requirement for push-pull pumping is the use of D1 resonant light which alternates between left and right circular polarization at the Bohr frequency of the state. The new pumping method works for a wide range of conditions, including atomic beams with almost no collisions, and atoms in buffer gases with pressures of many atmospheres.

  3. Charge asymmetry in pure vibrational states of the HD molecule

    NASA Astrophysics Data System (ADS)

    Bubin, Sergiy; Leonarski, Filip; Stanke, Monika; Adamowicz, Ludwik

    2009-03-01

    Very accurate variational calculations of all rotationless states (also called pure vibrational states) of the HD molecule have been performed within the framework that does not assume the Born-Oppenheimer (BO) approximation. The non-BO wave functions of the states describing the internal motion of the proton, the deuteron, and the two electrons were expanded in terms of one-center explicitly correlated Gaussian functions multiplied by even powers of the internuclear distance. Up to 6000 functions were used for each state. Both linear and nonlinear parameters of the wave functions of all 18 states were optimized with a procedure that employs the analytical gradient of the energy with respect to the nonlinear parameters of the Gaussians. These wave functions were used to calculate expectation values of the interparticle distances and some other related quantities. The results allow elucidation of the charge asymmetry in HD as a function of the vibrational excitation.

  4. Protecting a Solid-State Spin from Decoherence Using Dressed Spin States

    NASA Astrophysics Data System (ADS)

    Golter, D. Andrew; Baldwin, Thomas K.; Wang, Hailin

    2014-12-01

    We report experimental studies of dressing an electron spin in diamond with resonant and continuous microwave fields to protect the electron spin from magnetic fluctuations induced by the nuclear spin bath. We use optical coherent population trapping (CPT) to probe the energy level structure, optically induced spin transitions, and spin decoherence rates of the dressed spin states. Dressing an electron spin with resonant microwaves at a coupling rate near 1 MHz leads to a 50 times reduction in the linewidth of the spin transition underlying the CPT process, limited by transit-time broadening. Compared with dynamical decoupling, where effects of the bath are averaged out at specific times, the dressed spin state provides a continuous protection from decoherence.

  5. Spin state switching in iron coordination compounds

    PubMed Central

    Gaspar, Ana B; Garcia, Yann

    2013-01-01

    Summary The article deals with coordination compounds of iron(II) that may exhibit thermally induced spin transition, known as spin crossover, depending on the nature of the coordinating ligand sphere. Spin transition in such compounds also occurs under pressure and irradiation with light. The spin states involved have different magnetic and optical properties suitable for their detection and characterization. Spin crossover compounds, though known for more than eight decades, have become most attractive in recent years and are extensively studied by chemists and physicists. The switching properties make such materials potential candidates for practical applications in thermal and pressure sensors as well as optical devices. The article begins with a brief description of the principle of molecular spin state switching using simple concepts of ligand field theory. Conditions to be fulfilled in order to observe spin crossover will be explained and general remarks regarding the chemical nature that is important for the occurrence of spin crossover will be made. A subsequent section describes the molecular consequences of spin crossover and the variety of physical techniques usually applied for their characterization. The effects of light irradiation (LIESST) and application of pressure are subjects of two separate sections. The major part of this account concentrates on selected spin crossover compounds of iron(II), with particular emphasis on the chemical and physical influences on the spin crossover behavior. The vast variety of compounds exhibiting this fascinating switching phenomenon encompasses mono-, oligo- and polynuclear iron(II) complexes and cages, polymeric 1D, 2D and 3D systems, nanomaterials, and polyfunctional materials that combine spin crossover with another physical or chemical property. PMID:23504535

  6. Multiboson Correlation Interferometry with Arbitrary Single-Photon Pure States.

    PubMed

    Tamma, Vincenzo; Laibacher, Simon

    2015-06-19

    We provide a compact full description of multiboson correlation measurements of arbitrary order N in passive linear interferometers with arbitrary input single-photon pure states. This allows us to physically analyze the novel problem of multiboson correlation sampling at the output of random linear interferometers. Our results also describe general multiboson correlation landscapes for an arbitrary number of input single photons and arbitrary interferometers. In particular, we use two different schemes to demonstrate, respectively, arbitrary-order quantum beat interference and 100% visibility entanglement correlations even for input photons distinguishable in their frequencies. PMID:26196976

  7. Emergence of canonical ensembles from pure quantum states.

    PubMed

    Cho, Jaeyoon; Kim, M S

    2010-04-30

    We consider a system weakly interacting with a bath as a thermodynamic setting to establish a quantum foundation of statistical physics. It is shown that even if the composite system is initially in an arbitrary nonequilibrium pure quantum state, the unitary dynamics of a generic weak interaction almost always drives the subsystem into the canonical ensemble, in the usual sense of typicality. A crucial step is taken by assuming that the matrix elements of the interaction Hamiltonian have random phases, while their amplitudes are left unrestricted. PMID:20482093

  8. Thermal pure quantum states of many-particle systems

    NASA Astrophysics Data System (ADS)

    Hyuga, Masahiko; Sugiura, Sho; Sakai, Kazumitsu; Shimizu, Akira

    2014-09-01

    We generalize the thermal pure quantum (TPQ) formulation of statistical mechanics, in such a way that it is applicable to systems whose Hilbert space is infinite dimensional. Assuming particle systems, we construct the grand-canonical TPQ (gTPQ) state, which is the counterpart of the grand-canonical Gibbs state of the ensemble formulation. A single realization of the gTPQ state gives all quantities of statistical-mechanical interest, with exponentially small probability of error. This formulation not only sheds new light on quantum statistical mechanics but also is useful for practical computations. As an illustration, we apply it to the Hubbard model, on a one-dimensional (1D) chain and on a two-dimensional (2D) triangular lattice. For the 1D chain, our results agree well with the exact solutions over wide ranges of temperature, chemical potential, and the on-site interaction. For the 2D triangular lattice, for which exact results are unknown, we obtain reliable results over a wide range of temperature. We also find that finite-size effects are much smaller in the gTPQ state than in the canonical TPQ state. This also shows that in the ensemble formulation the grand-canonical Gibbs state of a finite-size system simulates an infinite system much better than the canonical Gibbs state.

  9. Chimera states in purely local delay-coupled oscillators

    NASA Astrophysics Data System (ADS)

    Bera, Bidesh K.; Ghosh, Dibakar

    2016-05-01

    We study the existence of chimera states in a network of locally coupled chaotic and limit-cycle oscillators. The necessary condition for chimera state in purely local coupled oscillators is discussed. At first, we numerically observe the existence of chimera or multichimera states in the locally coupled Hindmarsh-Rose neuron model. We find that delay time in the nonlinear local coupling reduces the domain of the coherent island in the parameter space of the synaptic coupling strength and time delay, and thus the coherent region can be completely eliminated once the time delay exceeds a certain threshold. We then consider another form of nonlinearity in the local coupling, and the existence of chimera states is observed in the time-delayed Mackey-Glass system and in a Van der Pol oscillator. We also discuss the effect of time delay in local coupling for the existence of chimera states in Mackey-Glass systems. The nonlinearity present in the coupling function plays a key role in the emergence of chimera or multichimera states. A phase diagram for the chimera state is identified over a wide parameter space.

  10. Monogamy of quantum correlations in three-qubit pure states

    NASA Astrophysics Data System (ADS)

    Sudha; Devi, A. R. Usha; Rajagopal, A. K.

    2012-01-01

    The limitation on the shareability of quantum entanglement over several parties, the so-called monogamy of entanglement, is an issue that has received considerable attention from the quantum information community over the last decade. A natural question of interest in this connection is whether monogamy of correlations is true for correlations other than entanglement. This issue is examined here by choosing quantum deficit, proposed by A. K. Rajagopal and R. W. Rendell [Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.66.022104 66, 022104 (2002)], an operational measure of correlations. In addition to establishing the polygamous nature of the class of three-qubit symmetric pure states characterized by two distinct Majorana spinors (to which the W states belong), those with three distinct Majorana spinors [to which Greenberger-Horne-Zeilinger (GHZ) states belong] are shown to either obey or violate monogamy relations. While the generalized W states can be monogamous or polygamous, the generalized GHZ states exhibit monogamy with respect to quantum deficit. The issue of using monogamy conditions based on quantum deficit to witness the states belonging to stochastic local operations and classical communication (SLOCC) inequivalent classes is discussed in light of these results.

  11. Passive interferometric symmetries of multimode Gaussian pure states

    NASA Astrophysics Data System (ADS)

    Gabay, Natasha; Menicucci, Nicolas C.

    2016-05-01

    As large-scale multimode Gaussian states begin to become accessible in the laboratory, their representation and analysis become a useful topic of research in their own right. The graphical calculus for Gaussian pure states provides powerful tools for their representation, while this work presents a useful tool for their analysis: passive interferometric (i.e., number-conserving) symmetries. Here we show that these symmetries of multimode Gaussian states simplify calculations in measurement-based quantum computing and provide constructive tools for engineering large-scale harmonic systems with specific physical properties, and we provide a general mathematical framework for deriving them. Such symmetries are generated by linear combinations of operators expressed in the Schwinger representation of U (2 ) , called nullifiers because the Gaussian state in question is a zero eigenstate of them. This general framework is shown to have applications in the noise analysis of continuous-various cluster states and is expected to have additional applications in future work with large-scale multimode Gaussian states.

  12. Explicit pure-state density operator structure for quantum tomography

    NASA Astrophysics Data System (ADS)

    Fan, Hong-yi; Lv, Cui-hong

    2009-10-01

    The formulation of region operators named by D. Ellinas and A. J. Bracken [Phys. Rev. A 78, 052106 (2008)], which appears as the phase-space integration corresponding to the straight line over the Wigner operator, is manifestly improved and generalized. By virtue of the technique of integration within ordered (both normally ordered and Weyl ordered) product of operators, we show that the integration involved in the generalized region operator can be directly carried through to completion that leads to the explicit pure-state density operator |u⟩λ,τλ,τ⟨u|, where |u⟩λ,τ makes up the coordinate-momentum intermediate representation. This directly results in that the tomogram of a quantum state |ψ⟩ is just proportional to |⟨u|ψ⟩λ,τ|2, where ⟨u|ψ⟩λ,τ is the wave function of |ψ⟩ in the coordinate-momentum intermediate representation.

  13. Analysis of optimal unambiguous discrimination of three pure quantum states

    NASA Astrophysics Data System (ADS)

    Ha, Donghoon; Kwon, Younghun

    2015-06-01

    We consider unambiguous discrimination of three pure quantum states. Necessary and sufficient conditions to decide which states should be detected for optimal measurement of unambiguous discrimination are provided in terms of inner products and the geometric phase Φ . We get the optimal measurement and the optimal failure probability when the optimal unambiguous discrimination does not require the detection of every given quantum state. When at least two quantum states are orthogonal to each other, we supply the optimal measurement and optimal failure probability in analytic form. When all three quantum states are not orthogonal to each other and Φ ≠0 , we find an analytic condition to determine the zero and nonzero elements for an optimal positive operator valued measure. We explain how to determine the solution in a geometric manner. Using the known solution of a case where the mutual inner products are real, we check the necessary and sufficient conditions when Φ =π and analyze the property of the singular point when Φ =0 and the relation between the optimal points.

  14. An Extended Equation of State Modeling Method I. Pure Fluids

    NASA Astrophysics Data System (ADS)

    Scalabrin, G.; Bettio, L.; Marchi, P.; Piazza, L.; Richon, D.

    2006-09-01

    A new technique is proposed here to represent the thermodynamic surface of a pure fluid in the fundamental Helmholtz energy form. The peculiarity of the present method is the extension of a generic equation of state for the target fluid, which is assumed as the basic equation, through the distortion of its independent variables by individual shape functions, which are represented by a neural network used as function approximator. The basic equation of state for the target fluid can have the simple functional form of a cubic equation, as, for instance, the Soave-Redlich-Kwong equation assumed in the present study. A set of nine fluids including hydrocarbons, haloalkane refrigerants, and strongly polar substances has been considered. For each of them the model has been regressed and then validated against volumetric and caloric properties generated in the vapor, liquid, and supercritical regions from highly accurate dedicated equations of state. In comparison with the underlying cubic equation of state, the prediction accuracy is improved by a factor between 10 and 100, depending on the property and on the region. It has been verified that about 100 density experimental points, together with from 10 to 20 coexistence data, are sufficient to guarantee high prediction accuracy for different thermodynamic properties. The method is a promising modeling technique for the heuristic development of multiparameter dedicated equations of state from experimental data.

  15. Spin state transitions in cobaltites: spectroscopic perspective

    NASA Astrophysics Data System (ADS)

    Hao Tjeng, Liu

    2010-03-01

    The class of cobalt-oxide based materials has attracted increasing interest in the last decade. A key aspect of the cobaltites that distinguishes them clearly from the Cu, Ni, and Mn oxides is the spin state degree of freedom of the Co3+ and Co4+ ions: the ions can be low spin, high spin, and perhaps even intermediate spin. This aspect comes on top of the orbital and charge degrees of freedom that already make the Cu, Ni, Mn systems so exciting. It is, however, also precisely this aspect that causes considerable debate in the literature. In this presentation we would like to show how synchrotron based soft-x-ray spectroscopies can successfully resolve the local electronic structure of the Co ions and thus contribute to a better understanding of the physical properties of the cobaltites. In particular, we will address the issue of spin state transitions, metal insulator transitions and the newly proposed spin-blockade phenomenon in several layered cobalt materials. --- Work done in collaboration with Z. Hu, M.W. Haverkort, C.F. Chang, H. Wu, T. Burnus, Y.Y. Chin, N. Hollmann, C. Schussler- Langeheine, M. Benomar, T. Lorenz, D.I. Khomskii (Univ. Cologne), A. Tanaka (Univ. Hiroshima), S.N. Barilo (NAS, Minsk), J. Cezar, N.B. Brookes (ESRF-Grenoble), H.H. Hsieh, H.J. Lin, C.T. Chen (NSRRC-Hsinchu). Supported by the DFG through SFB 608.

  16. Entanglement of three-qubit pure states in terms of teleportation capability

    SciTech Connect

    Lee, Soojoon; Joo, Jaewoo; Kim, Jaewan

    2005-08-15

    We define an entanglement measure, called the partial tangle, which represents the residual two-qubit entanglement of a three-qubit pure state. By its explicit calculations for three-qubit pure states, we show that the partial tangle is closely related to the faithfulness of a teleportation scheme over a three-qubit pure state.

  17. Antiferromagnetic Spin-S Chains with Exactly Dimerized Ground States

    NASA Astrophysics Data System (ADS)

    Michaud, Frédéric; Vernay, François; Manmana, Salvatore R.; Mila, Frédéric

    2012-03-01

    We show that spin S Heisenberg spin chains with an additional three-body interaction of the form (Si-1·Si)(Si·Si+1)+H.c. possess fully dimerized ground states if the ratio of the three-body interaction to the bilinear one is equal to 1/[4S(S+1)-2]. This result generalizes the Majumdar-Ghosh point of the J1-J2 chain, to which the present model reduces for S=1/2. For S=1, we use the density matrix renormalization group method to show that the transition between the Haldane and the dimerized phases is continuous with a central charge c=3/2. Finally, we show that such a three-body interaction appears naturally in a strong-coupling expansion of the Hubbard model, and we discuss the consequences for the dimerization of actual antiferromagnetic chains.

  18. Steady-state spin squeezing generation in diamond nanostructures

    NASA Astrophysics Data System (ADS)

    Ma, Yong-Hong; Zhang, Xue-Feng

    2014-04-01

    As one kind of many body entangled states, spin squeezed states can be used to implement the high precise measurement beyond the standard quantum limit. Inspired by the novel spin squeezing scheme based on phonon-induced spin-spin interactions [S. D. Bennett et al., Phys. Rev. Lett. 110, 156402 (2013), 10.1103/PhysRevLett.110.156402], we reexamine the steady-state behaviors for the spin ensemble in diamond nanostructures by exerting a controllable microwave field. By using the phase-space approach we calculate analytically fluctuations of collective spin operators. We find that there is bistability and spin squeezing for the steady-state spin ensemble, despite the mechanical damping considered. Moreover, our work shows that bistability and spin squeezing can be controlled by microwave field and Zeeman splitting. The present scheme can be used to increase the stability of spin clocks, magnetometers, and other measurements based on spin-spin interaction in diamond nanostructures.

  19. High Fidelity Symmetric Telecloning and Entanglement Distribution of Spin Quantum States by Weak Measurement and Reversal

    NASA Astrophysics Data System (ADS)

    Wang, Qiong; He, Zhi; Yao, Chun-Mei; Li, Wen-Juan

    2016-08-01

    We propose a physical realization of robust symmetric telecloning scheme for spin quantum states by employing the weak measurement and reversal (WMR) operation. Using proper WMR, the ultrahigh telecloning fidelity and long distance of quantum state transfer with certain success probability can be achieved. More interestingly, the lowest average telecloning fidelity can attain 80 %, which is almost independent of the spin chain length. We also study the properties of entanglement distribution via the spin chain for arbitrary two-qubit entangled pure states as inputs and find that the WMR operation indeed helps for protecting distributed entanglement.

  20. Geometric local invariants and pure three-qubit states

    SciTech Connect

    Williamson, Mark S.; Ericsson, Marie; Johansson, Markus; Sjoeqvist, Erik; Sudbery, Anthony; Vedral, Vlatko; Wootters, William K.

    2011-06-15

    We explore a geometric approach to generating local SU(2) and SL(2,C) invariants for a collection of qubits inspired by lattice gauge theory. Each local invariant or ''gauge'' invariant is associated with a distinct closed path (or plaquette) joining some or all of the qubits. In lattice gauge theory, the lattice points are the discrete space-time points, the transformations between the points of the lattice are defined by parallel transporters, and the gauge invariant observable associated with a particular closed path is given by the Wilson loop. In our approach the points of the lattice are qubits, the link transformations between the qubits are defined by the correlations between them, and the gauge invariant observable, the local invariants associated with a particular closed path, are also given by a Wilson looplike construction. The link transformations share many of the properties of parallel transporters, although they are not undone when one retraces one's steps through the lattice. This feature is used to generate many of the invariants. We consider a pure three-qubit state as a test case and find we can generate a complete set of algebraically independent local invariants in this way; however, the framework given here is applicable to generating local unitary invariants for mixed states composed of any number of d-level quantum systems. We give an operational interpretation of these invariants in terms of observables.

  1. Geometric local invariants and pure three-qubit states

    NASA Astrophysics Data System (ADS)

    Williamson, Mark S.; Ericsson, Marie; Johansson, Markus; Sjöqvist, Erik; Sudbery, Anthony; Vedral, Vlatko; Wootters, William K.

    2011-06-01

    We explore a geometric approach to generating local SU(2) and SL(2,C) invariants for a collection of qubits inspired by lattice gauge theory. Each local invariant or “gauge” invariant is associated with a distinct closed path (or plaquette) joining some or all of the qubits. In lattice gauge theory, the lattice points are the discrete space-time points, the transformations between the points of the lattice are defined by parallel transporters, and the gauge invariant observable associated with a particular closed path is given by the Wilson loop. In our approach the points of the lattice are qubits, the link transformations between the qubits are defined by the correlations between them, and the gauge invariant observable, the local invariants associated with a particular closed path, are also given by a Wilson looplike construction. The link transformations share many of the properties of parallel transporters, although they are not undone when one retraces one’s steps through the lattice. This feature is used to generate many of the invariants. We consider a pure three-qubit state as a test case and find we can generate a complete set of algebraically independent local invariants in this way; however, the framework given here is applicable to generating local unitary invariants for mixed states composed of any number of d-level quantum systems. We give an operational interpretation of these invariants in terms of observables.

  2. Solid State Physics View of Liquid State Chemistry III. Electrical Conductance of Pure and Impure Water

    NASA Astrophysics Data System (ADS)

    Binbin, Jie; Chihtang, Sah

    2014-04-01

    The ‘abnormally’ high electrical conductivity of pure water was recently studied by us using our protonic bond, trap and energy band model, with five host particles: the positive and negative protons, and the amphoteric protonic trap in three charge states, positive, neutral and negative. Our second report described the electrical charge storage capacitance of pure and impure water. This third report presents the theory of particle density and electrical conductance of pure and impure water, including the impuritons, which consist of an impurity ion bonded to a proton, proton-hole or proton trap and which significantly affect impure waters' properties.

  3. Temperature-dependent remote control of polarization and coherence intensity with sender's pure initial state

    NASA Astrophysics Data System (ADS)

    Fel'dman, E. B.; Kuznetsova, E. I.; Zenchuk, A. I.

    2016-06-01

    We study the remote creation of the polarization and intensity of the first-order coherence (or coherence intensity) in long spin-1/2 chains with one-qubit sender and receiver. Therewith we use a physically motivated initial condition with the pure state of the sender and the thermodynamical equilibrium state of the other nodes. The main part of the creatable region is a one-to-one map of the initial state (control) parameters, except the small subregion twice covered by the control parameters, which appears owing to the chosen initial state. The polarization and coherence intensity behave differently in the state creation process. In particular, the coherence intensity cannot reach any significant value unless the polarization is large in long chains (unlike the short ones), but the opposite is not true. The coherence intensity vanishes with an increase in the chain length, while the polarization (by absolute value) is not sensitive to this parameter. We represent several characteristics of the creatable polarization and coherence intensity and describe their relation to the parameters of the initial state. The link to the eigenvalue-eigenvector parametrization of the receiver's state space is given.

  4. Temperature-dependent remote control of polarization and coherence intensity with sender's pure initial state

    NASA Astrophysics Data System (ADS)

    Fel'dman, E. B.; Kuznetsova, E. I.; Zenchuk, A. I.

    2016-03-01

    We study the remote creation of the polarization and intensity of the first-order coherence (or coherence intensity) in long spin-1/2 chains with one-qubit sender and receiver. Therewith we use a physically motivated initial condition with the pure state of the sender and the thermodynamical equilibrium state of the other nodes. The main part of the creatable region is a one-to-one map of the initial state (control) parameters, except the small subregion twice covered by the control parameters, which appears owing to the chosen initial state. The polarization and coherence intensity behave differently in the state creation process. In particular, the coherence intensity cannot reach any significant value unless the polarization is large in long chains (unlike the short ones), but the opposite is not true. The coherence intensity vanishes with an increase in the chain length, while the polarization (by absolute value) is not sensitive to this parameter. We represent several characteristics of the creatable polarization and coherence intensity and describe their relation to the parameters of the initial state. The link to the eigenvalue-eigenvector parametrization of the receiver's state space is given.

  5. The geometric measure of entanglement for a symmetric pure state with non-negative amplitudes

    SciTech Connect

    Hayashi, Masahito; Markham, Damian; Owari, Masaki; Virmani, Shashank

    2009-12-15

    In this paper for a class of symmetric multiparty pure states, we consider a conjecture related to the geometric measure of entanglement: ''for a symmetric pure state, the closest product state in terms of the fidelity can be chosen as a symmetric product state.'' We show that this conjecture is true for symmetric pure states whose amplitudes are all non-negative in a computational basis. The more general conjecture is still open.

  6. Equation of state, initiation, and detonation of pure ammonium nitrate

    NASA Astrophysics Data System (ADS)

    Robbins, D. L.; Sheffield, S. A.; Dattelbaum, D. M.; Velisavljevic, N.; Stahl, D. B.

    2009-06-01

    Ammonium nitrate (AN) is a widely used fertilizer and mining explosive throughout the world. One of the more common explosives using AN is called ANFO, a mixture of AN prills and fuel oil in a 94:6 ratio by weight. The AN prills are specially made to absorb the fuel oil, forming a mixture that reacts under shock loading through a diffusion-controlled process, resulting in a non-ideal explosive with detonation velocities around 4 km/s. While there are a number of studies on ANFO, there are only a few studies relating to the equation of state (EOS) and detonation properties of pure AN - resulting mainly from studies of accidents that have occurred during transportation of large quantities of AN. We present the results of a series of gas gun-driven plate impact experiments on pressed AN ranging in density from 1.72 to 0.9 g/cm^3. Several of the high density experiments were performed in front surface impact geometry, in which pressed AN disks were built into the projectile front and impacted onto LiF windows. Additional experiments at low density have been done in ``half cell'' multiple magnetic gauge gun experiments. From this work a complete unreacted EOS has been developed, as well as some initiation and detonation information. Additional high pressure x-ray diffraction experiments in diamond anvil cells have provided a static isotherm for AN.

  7. Spin-split states in aromatic molecules

    SciTech Connect

    Hirsh, J.E. . Dept. of Physics)

    1990-06-01

    A state where spin currents exist in the absence of external fields has recently been proposed to describe the low-temperature phase of chromium. It is proposed here that such a state may also describe the ground of aromatic molecules. It is argued that this point of view provides a more natural explanation for the large diamagnetic susceptibilities and NMR shifts observed in these molecules than the conventional viewpoint. The authors model suggests a new memory mechanism.

  8. High-spin states in ^88Kr

    NASA Astrophysics Data System (ADS)

    Fotiades, N.; Lisetskiy, A. F.; Cizewski, J. A.; Krücken, R.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Becker, J. A.; Younes, W.

    2007-10-01

    High-spin states in ^88Kr have been studied following the fission of the ^226Th compound nucleus formed in a fusion-evaporation reaction (^18O at 91 MeV on ^208Pb). The Gammasphere array was used to detect γ-ray coincidences. High-spin states up to spin (14^+) and ˜8 MeV excitation energy have been established. The level scheme reported for ^88Kr in the spontaneous fission of ^248Cm [1] has been enriched and extended to higher spin and excitation energies. Differences between the level scheme reported in [1] and that obtained in the present work will be discussed. The observed experimental states are also compared with theoretical shell-model and interacting-boson-model-2 calculations. This work has been supported by the U.S. Department of Energy under Contracts No. DE-AC52-06NA25396 (LANL), W-7405-ENG-48 (LLNL) and AC03-76SF00098 (LBNL) and by the National Science Foundation (Rutgers). [1] T. Rzaca-Urban et al., Eur. Phys. J. A 9, 165 (2000).

  9. Spin transistor based on pure nonlocal Andreev reflection in EuO-graphene/superconductor/EuO-graphene nanostructure

    NASA Astrophysics Data System (ADS)

    Ang, Yee Sin; Ang, Lay Kee; Zhang, Chao; Ma, Zhongshui

    In graphene-magnetic-insulator hybrid structure such as graphene-Europium-oxide, proximity induced exchange interaction opens up a spin-dependent bandgap and spin splitting in the Dirac band. We show that such band topology allows pure crossed Andreev reflection to be generated exclusively without the parasitic local Andreev reflection and elastic cotunnelling over a wide range of bias and Fermi levels. We model the charge transport in an EuO-graphene/superconductor/EuO-graphene three-terminal device and found that the pure non-local conductance exhibits rapid on/off switching characteristic with a minimal subthreshold swing of ~ 20 mV. Non-local conductance oscillation is observed when the Fermi levels in the superconducting lead is varied. The oscillatory behavior is directly related to the quasiparticle propagation in the superconducting lead and hence can be used as a tool to probe the subgap quasiparticle mode in superconducting graphene. The non-local current is 100% spin-polarized and is highly tunable in our proposed device. This opens up the possibility of highly tunable graphene-based spin transistor that operates purely in the non-local transport regime.

  10. Random pure states: Quantifying bipartite entanglement beyond the linear statistics

    NASA Astrophysics Data System (ADS)

    Vivo, Pierpaolo; Pato, Mauricio P.; Oshanin, Gleb

    2016-05-01

    We analyze the properties of entangled random pure states of a quantum system partitioned into two smaller subsystems of dimensions N and M . Framing the problem in terms of random matrices with a fixed-trace constraint, we establish, for arbitrary N ≤M , a general relation between the n -point densities and the cross moments of the eigenvalues of the reduced density matrix, i.e., the so-called Schmidt eigenvalues, and the analogous functionals of the eigenvalues of the Wishart-Laguerre ensemble of the random matrix theory. This allows us to derive explicit expressions for two-level densities, and also an exact expression for the variance of von Neumann entropy at finite N ,M . Then, we focus on the moments E {Ka} of the Schmidt number K , the reciprocal of the purity. This is a random variable supported on [1 ,N ] , which quantifies the number of degrees of freedom effectively contributing to the entanglement. We derive a wealth of analytical results for E {Ka} for N =2 and 3 and arbitrary M , and also for square N =M systems by spotting for the latter a connection with the probability P (xminGUE≥√{2 N }ξ ) that the smallest eigenvalue xminGUE of an N ×N matrix belonging to the Gaussian unitary ensemble is larger than √{2 N }ξ . As a by-product, we present an exact asymptotic expansion for P (xminGUE≥√{2 N }ξ ) for finite N as ξ →∞ . Our results are corroborated by numerical simulations whenever possible, with excellent agreement.

  11. Random pure states: Quantifying bipartite entanglement beyond the linear statistics.

    PubMed

    Vivo, Pierpaolo; Pato, Mauricio P; Oshanin, Gleb

    2016-05-01

    We analyze the properties of entangled random pure states of a quantum system partitioned into two smaller subsystems of dimensions N and M. Framing the problem in terms of random matrices with a fixed-trace constraint, we establish, for arbitrary N≤M, a general relation between the n-point densities and the cross moments of the eigenvalues of the reduced density matrix, i.e., the so-called Schmidt eigenvalues, and the analogous functionals of the eigenvalues of the Wishart-Laguerre ensemble of the random matrix theory. This allows us to derive explicit expressions for two-level densities, and also an exact expression for the variance of von Neumann entropy at finite N,M. Then, we focus on the moments E{K^{a}} of the Schmidt number K, the reciprocal of the purity. This is a random variable supported on [1,N], which quantifies the number of degrees of freedom effectively contributing to the entanglement. We derive a wealth of analytical results for E{K^{a}} for N=2 and 3 and arbitrary M, and also for square N=M systems by spotting for the latter a connection with the probability P(x_{min}^{GUE}≥sqrt[2N]ξ) that the smallest eigenvalue x_{min}^{GUE} of an N×N matrix belonging to the Gaussian unitary ensemble is larger than sqrt[2N]ξ. As a by-product, we present an exact asymptotic expansion for P(x_{min}^{GUE}≥sqrt[2N]ξ) for finite N as ξ→∞. Our results are corroborated by numerical simulations whenever possible, with excellent agreement. PMID:27300829

  12. Spin-state chemistry of deuterated ammonia

    NASA Astrophysics Data System (ADS)

    Sipilä, O.; Harju, J.; Caselli, P.; Schlemmer, S.

    2015-09-01

    Aims: We aim to develop a chemical model that contains a consistent description of spin-state chemistry in reactions involving chemical species with multiple deuterons. We apply the model to the specific case of deuterated ammonia, to derive values for the various spin-state ratios. Methods: We applied symmetry rules in the context of the complete scrambling assumption to calculate branching ratio tables for reactions between chemical species that include multiple protons and/or deuterons. New reaction sets for both gas-phase and grain-surface chemistry were generated using an automated routine that forms all possible spin-state variants of any given reaction with up to six H/D atoms, using the predetermined branching ratios. Both a single-point and a modified Bonnor-Ebert model were considered to study the density and temperature dependence of ammonia and its isotopologs, and the associated spin-state ratios. Results: We find that the spin-state ratios of the ammonia isotopologs are, at late times, very different from their statistical values. The ratios are rather insensitive to variations in the density, but present strong temperature dependence. We derive high peak values (~0.1) for the deuterium fraction in ammonia, in agreement with previous (gas-phase) models. The deuterium fractionation is strongest at high density, corresponding to a high degree of depletion, and also presents temperature dependence. We find that in the temperature range 5 K to 20 K, the deuterium fractionation peaks at ~15 K, while most of the ortho/para (and meta/para for ND3) ratios present a minimum at 10 K (ortho/para NH2D has instead a maximum at this temperature). Conclusions: Owing to the density and temperature dependence found in the abundances and spin-state ratios of ammonia and its isotopologs, it is evident that observations of ammonia and its deuterated forms can provide important constraints on the physical structure of molecular clouds. Appendix A is available in

  13. Optimal pulse spacing for dynamical decoupling in the presence of a purely dephasing spin bath

    SciTech Connect

    Ajoy, Ashok; Alvarez, Gonzalo A.; Suter, Dieter

    2011-03-15

    Maintaining quantum coherence is a crucial requirement for quantum computation; hence protecting quantum systems against their irreversible corruption due to environmental noise is an important open problem. Dynamical decoupling (DD) is an effective method for reducing decoherence with a low control overhead. It also plays an important role in quantum metrology, where, for instance, it is employed in multiparameter estimation. While a sequence of equidistant control pulses [the Carr-Purcell-Meiboom-Gill (CPMG) sequence] has been ubiquitously used for decoupling, Uhrig recently proposed that a nonequidistant pulse sequence [the Uhrig dynamic decoupling (UDD) sequence] may enhance DD performance, especially for systems where the spectral density of the environment has a sharp frequency cutoff. On the other hand, equidistant sequences outperform UDD for soft cutoffs. The relative advantage provided by UDD for intermediate regimes is not clear. In this paper, we analyze the relative DD performance in this regime experimentally, using solid-state nuclear magnetic resonance. Our system qubits are {sup 13}C nuclear spins and the environment consists of a {sup 1}H nuclear spin bath whose spectral density is close to a normal (Gaussian) distribution. We find that in the presence of such a bath, the CPMG sequence outperforms the UDD sequence. An analogy between dynamical decoupling and interference effects in optics provides an intuitive explanation as to why the CPMG sequence performs better than any nonequidistant DD sequence in the presence of this kind of environmental noise.

  14. Canonical form of three-fermion pure-states with six single particle states

    SciTech Connect

    Chen, Lin; Ž Ðoković, Dragomir; Grassl, Markus; Zeng, Bei

    2014-08-01

    We construct a canonical form for pure states in Λ³(C⁶), the three-fermion system with six single particle states, under local unitary (LU) transformations, i.e., the unitary group U(6). We also construct a minimal set of generators of the algebra of polynomial U(6)-invariants on Λ³(C⁶). It turns out that this algebra is isomorphic to the algebra of polynomial LU-invariants of three-qubits which are additionally invariant under qubit permutations. As a consequence of this surprising fact, we deduce that there is a one-to-one correspondence between the U(6)-orbits of pure three-fermion states in Λ³(C⁶) and the LU orbits of pure three-qubit states when qubit permutations are allowed. As an important byproduct, we obtain a new canonical form for pure three-qubit states under LU transformations U(2) × U(2) × U(2) (no qubit permutations allowed)

  15. Spin-orbit states of neutron wave packets

    NASA Astrophysics Data System (ADS)

    Nsofini, Joachim; Sarenac, Dusan; Wood, Christopher J.; Cory, David G.; Arif, Muhammad; Clark, Charles W.; Huber, Michael G.; Pushin, Dmitry A.

    2016-07-01

    We propose a method to prepare an entangled spin-orbit state between the spin and the orbital angular momenta of a neutron wave packet. This spin-orbit state is created by passing neutrons through the center of a quadrupole magnetic field, which provides a coupling between the spin and orbital degrees of freedom. A Ramsey-fringe-type measurement is suggested as a means of verifying the spin-orbit correlations.

  16. Complete solution for unambiguous discrimination of three pure states with real inner products

    SciTech Connect

    Sugimoto, H.; Hashimoto, T.; Horibe, M.; Hayashi, A.

    2010-09-15

    Complete solutions are given in a closed analytic form for unambiguous discrimination of three general pure states with real mutual inner products. For this purpose, we first establish some general results on unambiguous discrimination of n linearly independent pure states. The uniqueness of solution is proved. The condition under which the problem is reduced to an (n-1)-state problem is clarified. After giving the solution for three pure states with real mutual inner products, we examine some difficulties in extending our method to the case of complex inner products. There is a class of set of three pure states with complex inner products for which we obtain an analytical solution.

  17. Four-state ferroelectric spin-valve

    PubMed Central

    Quindeau, Andy; Fina, Ignasi; Marti, Xavi; Apachitei, Geanina; Ferrer, Pilar; Nicklin, Chris; Pippel, Eckhard; Hesse, Dietrich; Alexe, Marin

    2015-01-01

    Spin-valves had empowered the giant magnetoresistance (GMR) devices to have memory. The insertion of thin antiferromagnetic (AFM) films allowed two stable magnetic field-induced switchable resistance states persisting in remanence. In this letter, we show that, without the deliberate introduction of such an AFM layer, this functionality is transferred to multiferroic tunnel junctions (MFTJ) allowing us to create a four-state resistive memory device. We observed that the ferroelectric/ferromagnetic interface plays a crucial role in the stabilization of the exchange bias, which ultimately leads to four robust electro tunnel electro resistance (TER) and tunnel magneto resistance (TMR) states in the junction. PMID:25961513

  18. Coulomb energy averaged over the nl{sup N}-atomic states with a definite spin

    SciTech Connect

    Kibler, M.; Smirnov, Yu. F.

    1995-03-05

    A purely group-theoretical approach (for which the symmetric group plays a central role), based upon the use of properties of fractional-parentage coefficients and isoscalar factors, is developed for the derivation of the Coulomb energy averaged over the states, with a definite spin, arising from an atomic configuration nl{sup N}. 15 refs.

  19. Typical pure states and the analysis of nonequilibrium processes of mesoscopic systems

    NASA Astrophysics Data System (ADS)

    Monnai, Takaaki; Sugita, Ayumu

    2016-05-01

    For isolated quantum many-body systems, we extend the availability of the intrinsic thermal nature of typical pure states to a class of nonequilibrium processes which start from an initial equilibrium. For concreteness, we calculate the spectral distribution of the work done on the system on the basis of a single pure state. It means that we can accurately calculate the entire fluctuation of the energy only from a single pure state instead of the thermodynamic ensembles.

  20. Spin State Estimation of Tumbling Small Bodies

    NASA Astrophysics Data System (ADS)

    Olson, Corwin; Russell, Ryan P.; Bhaskaran, Shyam

    2016-06-01

    It is expected that a non-trivial percentage of small bodies that future missions may visit are in non-principal axis rotation (i.e. "tumbling"). The primary contribution of this paper is the application of the Extended Kalman Filter (EKF) Simultaneous Localization and Mapping (SLAM) method to estimate the small body spin state, mass, and moments of inertia; the spacecraft position and velocity; and the surface landmark locations. The method uses optical landmark measurements, and an example scenario based on the Rosetta mission is used. The SLAM method proves effective, with order of magnitude decreases in the spacecraft and small body spin state errors after less than a quarter of the comet characterization phase. The SLAM method converges nicely for initial small body angular velocity errors several times larger than the true rates (effectively having no a priori knowledge of the angular velocity). Surface landmark generation and identification are not treated in this work, but significant errors in the initial body-fixed landmark positions are effectively estimated. The algorithm remains effective for a range of different truth spin states, masses, and center of mass offsets that correspond to expected tumbling small bodies throughout the solar system.

  1. Spin State Estimation of Tumbling Small Bodies

    NASA Astrophysics Data System (ADS)

    Olson, Corwin; Russell, Ryan P.; Bhaskaran, Shyam

    2016-02-01

    It is expected that a non-trivial percentage of small bodies that future missions may visit are in non-principal axis rotation (i.e. "tumbling"). The primary contribution of this paper is the application of the Extended Kalman Filter (EKF) Simultaneous Localization and Mapping (SLAM) method to estimate the small body spin state, mass, and moments of inertia; the spacecraft position and velocity; and the surface landmark locations. The method uses optical landmark measurements, and an example scenario based on the Rosetta mission is used. The SLAM method proves effective, with order of magnitude decreases in the spacecraft and small body spin state errors after less than a quarter of the comet characterization phase. The SLAM method converges nicely for initial small body angular velocity errors several times larger than the true rates (effectively having no a priori knowledge of the angular velocity). Surface landmark generation and identification are not treated in this work, but significant errors in the initial body-fixed landmark positions are effectively estimated. The algorithm remains effective for a range of different truth spin states, masses, and center of mass offsets that correspond to expected tumbling small bodies throughout the solar system.

  2. Exact coherent states in purely elastic parallel shear flows

    NASA Astrophysics Data System (ADS)

    Searle, Toby; Morozov, Alexander

    2014-11-01

    Parallel shear flows provide a model system for the understanding of the transition to and structure of incompressible Newtonian turbulence. The turbulent attractor is often thought of as structured by a series of exact solutions to the Navier-Stokes equations, where a turbulent flow ``pinballs'' between these solutions in phase space. The most intuitive mechanism for the appearance of these structures was formulated by F. Waleffe and is known as ``the self-sustaining process.'' A novel form of turbulence has been discovered in polymeric fluids where the Reynold's number is low, Re < 1 , and the Weissenberg number (characterising the fluid elasticity) is large. Using an analogy with the Newtonian self-sustaining process, we attempt to construct the purely elastic counterpart for plane Couette flow of polymer solutions. By introducing a forcing term to the coupled Navier-Stokes and Oldroyd-B equations, we observe the formation of purely elastic streaks and consider their linear stability. We find that there exists a previously unrecognised purely elastic analogue of the Kelvin-Helmholtz instability that gives rise to the streamwise waviness of Newtonian coherent structures. We discuss how this instability might close the cycle and lead to a sustained purely elastic coherent structure. SUPA, School of Physics and Astronomy, University of Edinburgh, Mayfield Road, Edinburgh, EH9 3JZ, UK.

  3. Bidirectional teleportation of a pure EPR state by using GHZ states

    NASA Astrophysics Data System (ADS)

    Hassanpour, Shima; Houshmand, Monireh

    2016-02-01

    In the present paper, a novel bidirectional quantum teleportation protocol is proposed. By using entanglement swapping technique, two GHZ states are shared as a quantum channel between Alice and Bob as legitimate users. In this scheme, based on controlled-not operation, single-qubit measurement, and appropriate unitary operations, two users can simultaneously transmit a pure EPR state to each other, While, in the previous protocols, the users can just teleport a single-qubit state to each other via more than four-qubit state. Therefore, the proposed scheme is economical compared with previous protocols.

  4. Coexistence of pure and mixed states in nonlinear maps

    NASA Astrophysics Data System (ADS)

    Roth, Yehuda

    2015-09-01

    Coherence and interaction are important concepts in physics. While interaction describes a relation between individual objects such as forces acting between distinguishable particles, coherent objects exist with the sole purpose of describing a single object. For example, each component of a vector provides us with only partial information. The whole picture is revealed only when the components are coherently related to their generating vector. Another example is a singlet of two spin ½- particles. The true nature of these two coherent particles is described by a spin-less single particle. Apparently it seems that objects can be either coherent or lion-coherent but they cannot be both simultaneously. This is almost true. We show that a system can be described simultaneously as coherent and lion-coherent but an observer can distinguish only one concept at a time.

  5. Spectroscopy of composite solid-state spin environments for improved metrology with spin ensembles

    NASA Astrophysics Data System (ADS)

    Bar-Gill, Nir; Pham, Linh; Belthangady, Chinmay; Lesage, David; Cappellaro, Paola; Maze, Jeronimo; Lukin, Mikhail; Yacoby, Amir; Walsworth, Ronald

    2012-02-01

    For precision coherent measurements with ensembles of quantum spins the relevant Figure-of-Merit (FOM) is the product of spin density and coherence lifetime, which is generally limited by the dynamics of spin coupling to the environment. Significant effort has been invested in understanding the causes of decoherence in a diverse range of spin systems in order to increase the FOM and improve measurement sensitivity. Here, we apply a coherent spectroscopic technique to characterize the dynamics of a composite solid-state spin environment consisting of Nitrogen-Vacancy (NV) color centers in room temperature diamond coupled to baths of electronic spin (N) and nuclear spin (13C) impurities. For diamond samples with a wide range of NV densities and impurity spin concentrations we employ a dynamical decoupling technique to minimize coupling to the environment, and find similar values for the FOM, which is three orders of magnitude larger than previously achieved in any room-temperature solid-state spin system, and thus should enable greatly improved precision spin metrology. We also identify a suppression of electronic spin bath dynamics in the presence of a nuclear spin bath of sufficient nuclear spin concentration. This suppression could inform efforts to engineer samples with even larger FOM for solid-state spin ensemble metrology and collective quantum information processing.

  6. Correlations and Werner states in finite spin linear arrays

    NASA Astrophysics Data System (ADS)

    Wells, P. R.; Chaves, C. M.; d'Albuquerque e Castro, J.; Koiller, Belita

    2013-10-01

    Pairwise quantum correlations in the ground state of an N-spins antiferromagnetic Heisenberg chain are investigated. By varying the exchange coupling between two neighboring sites, it is possible to reversibly drive spins from entangled to disentangled states. For even N, the two-spin density matrix is written in the form of a Werner state, allowing identification of its single parameter with the usual spin-spin correlation function. The N = 4 chain is identified as a promising system for practical demonstrations of non-classical correlations and the realization of Werner states in familiar condensed matter systems. Fabrication and measurement ingredients are within current capabilities.

  7. Generation of pure spin currents via Auger recombination in quantum wells with Rashba splitting

    SciTech Connect

    Afanasiev, A. N. Greshnov, A. A. Greshnov, A. A.

    2015-10-15

    We propose a nonoptical mechanism for generating spin current via Auger recombination in semiconductor quantum wells (QWs) with spin–orbit splitting associated with structural QW asymmetry. It is shown that Auger recombination in narrow-bandgap semiconductors makes it possible to produce spin currents that exceed those that are obtained in the case of intraband as well as interband optical excitation. Analysis shows that the interference term in the expression for the Auger-recombination rate is responsible for the generation of spin currents.

  8. The tumbling spin state of (99942) Apophis

    NASA Astrophysics Data System (ADS)

    Pravec, P.; Scheirich, P.; Ďurech, J.; Pollock, J.; Kušnirák, P.; Hornoch, K.; Galád, A.; Vokrouhlický, D.; Harris, A. W.; Jehin, E.; Manfroid, J.; Opitom, C.; Gillon, M.; Colas, F.; Oey, J.; Vraštil, J.; Reichart, D.; Ivarsen, K.; Haislip, J.; LaCluyze, A.

    2014-05-01

    Our photometric observations of Asteroid (99942) Apophis from December 2012 to April 2013 revealed it to be in a state of non-principal axis rotation (tumbling). We constructed its spin and shape model and found that it is in a moderately excited Short Axis Mode (SAM) state with a ratio of the rotational kinetic energy to the basic spin state energy E/E0=1.024±0.013. (All quoted uncertainties correspond to 3σ.) The greatest and intermediate principal moments of inertia are nearly the same with I2/I3=0.965-0.015+0.009, but the smallest principal moment of inertia is substantially lower with I1/I3=0.61-0.08+0.11; the asteroid’s dynamically equivalent ellipsoid is close to a prolate ellipsoid. The precession and rotation periods are Pϕ=27.38±0.07 h and Pψ=263±6 h, respectively; the strongest observed lightcurve amplitude for the SAM case is in the 2nd harmonic of P1=P=30.56±0.01 h. The rotation is retrograde with the angular momentum vector’s ecliptic longitude and latitude of 250° and -75° (the uncertainty area is approximately an ellipse with the major and minor semiaxes of 27° and 14°, respectively). An implication of the retrograde rotation is a somewhat increased probability of the Apophis’ impact in 2068, but it is still very small with the risk level on the Palermo Scale remaining well below zero. Apophis is a member of the population of slowly tumbling asteroids. Applying the theory of asteroid nutational damping by Breiter et al. (Breiter, S., Rożek, A., Vokrouhlický, D. [2012]. Mon. Not. R. Astron. Soc. 427, 755-769), we found that slowly tumbling asteroids predominate in the spin rate-size range where their estimated damping times are greater than about 0.2 Gyr. The appearance that the PA/NPA rotators transition line seems to follow a line of constant damping time may be because there are two or more asteroid spin evolution mechanisms in play, or the factor of μQ (the elastic modulus times the quality factor) is not constant but it may

  9. Observables can be tailored to change the entanglement of any pure state

    SciTech Connect

    Harshman, N. L.; Ranade, Kedar S.

    2011-07-15

    We show that, for a finite-dimensional Hilbert space, there exist observables that induce a tensor product structure such that the entanglement properties of any pure state can be tailored. In particular, we provide an explicit, finite method for constructing observables in an unstructured d-dimensional system so that an arbitrary known pure state has any Schmidt decomposition with respect to an induced bipartite tensor product structure. In effect, this article demonstrates that, in a finite-dimensional Hilbert space, entanglement properties can always be shifted from the state to the observables and all pure states are equivalent as entanglement resources in the ideal case of complete control of observables.

  10. Concurrence of assistance and Mermin inequality on three-qubit pure states

    SciTech Connect

    Chi, Dong Pyo; Kim, Taewan; Lee, Kyungjin; Jeong, Kabgyun; Lee, Soojoon

    2010-04-15

    We study a relation between the concurrence of assistance and the Mermin inequality on three-qubit pure states and claim that if a three-qubit pure state has a minimal concurrence of assistance greater than 1/2 then the state violates some Mermin inequality. In this work, we analytically show that our claim holds for several classes and also find that it can be generalized to the set of all three-qubit pure states by exploiting previous numerical work [C. Emary and C. W. J. Beenakker, Phys. Rev. A 69, 032317 (2004)].

  11. Neutron 2 p and 1 f spin-orbit splittings in 40Ca,36S , and 34Si N =20 isotones: Tensor-induced and pure spin-orbit effects

    NASA Astrophysics Data System (ADS)

    Grasso, M.; Anguiano, M.

    2015-11-01

    Neutron 2 p and 1 f spin-orbit splittings were recently measured in the isotones 37S and 35Si by (d ,p ) transfer reactions. Values were reported by using the major fragments of the states. An important reduction of the p splitting was observed, from 37S to 35Si , associated with a strong modification of the spin-orbit potential in the central region of the nucleus 35Si . We analyze 2 p and 1 f neutron spin-orbit splittings in the N =20 isotones 40Ca,36S , and 34Si . We employ several Skyrme and Gogny interactions to reliably isolate pure spin-orbit and tensor-induced contributions, within the mean-field approximation. We use interactions (i) without the tensor force, (ii) with the tensor force and with tensor parameters adjusted on top of existing parametrizations, nd (iii) with the tensor force and with tensor and spin-orbit parameters adjusted simultaneously on top of existing parametrizations. We predict in cases (ii) and (iii) a non-negligible reduction of both p and f splittings, associated with neutron-proton tensor effects, from 40Ca to 36S . The two splittings are further decreased for the three types of interactions, going from 36S to 34Si . This reduction is produced by the spin-orbit force and is not affected by tensor-induced contributions. For both reductions, from 40Ca to 36S and from 36S to 34Si , we predict in all cases that the modification is more pronounced for p than for f splittings. The measurement of the centroids for neutron 2 p and 1 f states in the nuclei 36S and 34Si would be interesting to validate this prediction experimentally. We show the importance of using interactions of type (iii), because they provide p and f splittings in the nucleus 40Ca which are in agreement with the corresponding experimental values.

  12. Exact results for the spin-1 Ising model on pure "square" Husimi lattices: Critical temperatures and spontaneous magnetization

    NASA Astrophysics Data System (ADS)

    Jurčišinová, E.; Jurčišin, M.

    2016-02-01

    We investigate the second order phase transitions of the ferromagnetic spin-1 Ising model on pure Husimi lattices built up from elementary squares with arbitrary values of the coordination number. It is shown that the critical temperatures of the second order phase transitions are driven by a single equation simultaneously on all such lattices. It is also shown that for arbitrary given value of the coordination number this equation is equivalent to the corresponding polynomial equation. The explicit form of these polynomial equations is present for the lattices with the coordination numbers z = 4 , 6, and 8. It is proven that, at least for the small values of the coordination number, the positions of the critical temperatures are uniquely determined. In addition, it is shown that the properties of all phases of the model are also driven by the corresponding single equations simultaneously on all pure Husimi lattices built up from elementary squares. The spontaneous magnetization of the model is investigated in detail.

  13. Universally coupled massive gravity, III: dRGT-Maheshwari pure spin-2, Ogievetsky-Polubarinov and arbitrary mass terms

    NASA Astrophysics Data System (ADS)

    Pitts, J. Brian

    2016-02-01

    Einstein's equations were derived for a free massless spin-2 field using universal coupling in the 1950-1970s by various authors; total stress-energy including gravity's served as a source for linear free field equations. A massive variant was likewise derived in the late 1960s by Freund, Maheshwari and Schonberg, and thought to be unique. How broad is universal coupling? In the last decade four 1-parameter families of massive spin-2 theories (contravariant, covariant, tetrad, and cotetrad of almost any density weights) have been derived using universal coupling. The (co)tetrad derivations included 2 of the 3 pure spin-2 theories due to de Rham, Gabadadze, and Tolley; those two theories first appeared in the 2-parameter Ogievetsky-Polubarinov family (1965), which developed the symmetric square root of the metric as a nonlinear group realization. One of the two theories was identified as pure spin-2 by Maheshwari in 1971-1972, thus evading the Boulware-Deser-Tyutin-Fradkin ghost by the time it was announced. Unlike the previous 4 families, this paper permits nonlinear field redefinitions to build the effective metric. By not insisting in advance on knowing the observable significance of the graviton potential to all orders, one finds that an arbitrary graviton mass term can be derived using universal coupling. The arbitrariness of a universally coupled mass/self-interaction term contrasts sharply with the uniqueness of the Einstein kinetic term. One might have hoped to use universal coupling as a tie-breaking criterion for choosing among theories that are equally satisfactory on more crucial grounds (such as lacking ghosts and having a smooth massless limit). But the ubiquity of universal coupling implies that the criterion does not favor any particular theories among those with the Einstein kinetic term.

  14. Optical Polarization Möbius Strips and Points of Purely Transverse Spin Density

    NASA Astrophysics Data System (ADS)

    Bauer, Thomas; Neugebauer, Martin; Leuchs, Gerd; Banzer, Peter

    2016-07-01

    Tightly focused light beams can exhibit complex and versatile structured electric field distributions. The local field may spin around any axis including a transverse axis perpendicular to the beams' propagation direction. At certain focal positions, the corresponding local polarization ellipse can even degenerate into a perfect circle, representing a point of circular polarization or C point. We consider the most fundamental case of a linearly polarized Gaussian beam, where—upon tight focusing—those C points created by transversely spinning fields can form the center of 3D optical polarization topologies when choosing the plane of observation appropriately. Because of the high symmetry of the focal field, these polarization topologies exhibit nontrivial structures similar to Möbius strips. We use a direct physical measure to find C points with an arbitrarily oriented spinning axis of the electric field and experimentally investigate the fully three-dimensional polarization topologies surrounding these C points by exploiting an amplitude and phase reconstruction technique.

  15. Pure-state tomography with the expectation value of Pauli operators

    NASA Astrophysics Data System (ADS)

    Ma, Xian; Jackson, Tyler; Zhou, Hui; Chen, Jianxin; Lu, Dawei; Mazurek, Michael D.; Fisher, Kent A. G.; Peng, Xinhua; Kribs, David; Resch, Kevin J.; Ji, Zhengfeng; Zeng, Bei; Laflamme, Raymond

    2016-03-01

    We examine the problem of finding the minimum number of Pauli measurements needed to uniquely determine an arbitrary n -qubit pure state among all quantum states. We show that only 11 Pauli measurements are needed to determine an arbitrary two-qubit pure state compared to the full quantum state tomography with 16 measurements, and only 31 Pauli measurements are needed to determine an arbitrary three-qubit pure state compared to the full quantum state tomography with 64 measurements. We demonstrate that our protocol is robust under depolarizing error with simulated random pure states. We experimentally test the protocol on two- and three-qubit systems with nuclear magnetic resonance techniques. We show that the pure-state tomography protocol saves us a number of measurements without considerable loss of fidelity. We compare our protocol with same-size sets of randomly selected Pauli operators and find that our selected set of Pauli measurements significantly outperforms those random sampling sets. As a direct application, our scheme can also be used to reduce the number of settings needed for pure-state tomography in quantum optical systems.

  16. Negative Correlations and Entanglement in Higher-Spin Dicke States

    NASA Astrophysics Data System (ADS)

    Wang, Xiaoqian; Zhong, Wei; Wang, Xiaoguang

    2016-06-01

    We consider entanglement criteria based on the spin squeezing inequalities for arbitrary spin systems. Here we use the negative correlations to detect the entanglement in the system with exchange symmetry. For arbitrary spin systems, we can find that the state is entangled, when the minimal pairwise correlation is negative. Then we give a parameter which is defined by the collective angular momentum operator, to detect the entanglement for the Dicke state with N spin -1 particles, and the results are as the same as negative correlation. We also consider the directions of negative correlation, the state is entangled in two orthogonal directions for the superposition of Dicke state without parity.

  17. Spin relaxation of iron in mixed state hemoproteins.

    PubMed Central

    Wajnberg, E; Kalinowski, H J; Bemski, G; Helman, J S

    1986-01-01

    In hemoproteins the relaxation mechanism of iron is Orbach for high spin (HS) and Raman for low spin (LS). We found that in met-hemoglobin and met-myoglobin, under conditions in which the two spin states coexist, both the HS and the LS states relax to the lattice through Orbach-like processes. Alos, very short (approximately 1 ns) and temperature independent transverse relaxation times T2 were estimated. This may result from the unusual electronic structure of mixed states hemoproteins that allows thermal equilibrium and interconversion of the spin states. PMID:3013333

  18. Low-energy-state dynamics of entanglement for spin systems

    SciTech Connect

    Jafari, R.

    2010-11-15

    We develop the ideas of the quantum renormalization group and quantum information by exploring the low-energy-state dynamics of entanglement resources of a system close to its quantum critical point. We demonstrate that low-energy-state dynamical quantities of one-dimensional magnetic systems can show a quantum phase transition point and show scaling behavior in the vicinity of the transition point. To present our idea, we study the evolution of two spin entanglements in the one-dimensional Ising model in the transverse field. The system is initialized as the so-called thermal ground state of the pure Ising model. We investigate the evolution of the generation of entanglement with increasing magnetic field. We obtain that the derivative of the time at which the entanglement reaches its maximum with respect to the transverse field diverges at the critical point and its scaling behaviors versus the size of the system are the same as the static ground-state entanglement of the system.

  19. Influences of Initial States on Entanglement Dynamics of Two Central Spins in a Spin Environment

    NASA Astrophysics Data System (ADS)

    Yu, Wen-Jian; Xu, Bao-Ming; Li, Lin; Zou, Jian; Li, Hai; Shao, Bin

    2016-03-01

    We investigate the entanglement dynamics of two electronic spins coupled to a bath of nuclear spins for two special cases, one is that two central spins both interact with a common bath, and the other is that one of two spins interacts with a bath. We consider three types of initial states with different correlations between the system and the bath, i.e., quantum correlation, classical correlation, and no-correlation. We show that the initial correlations (no matter quantum correlations or classical correlations) can effectively avoid the occurrence of entanglement sudden death. Irrespective of whether both two spins or only one of the two spins interacts with the bath, the system can gain more entanglement in the process of the time evolution for initial quantum correlations. In addition, we find that the effects of the distribution of coupling constants on entanglement dynamics crucially depend on the initial state of the spin bath.

  20. Systematic generation of entanglement measures for pure states

    NASA Astrophysics Data System (ADS)

    Sugita, Ayumu

    2008-05-01

    We propose a method to generate entanglement measures systematically by using the irreducible decomposition of some copies of a state under the local unitary (LU) transformations. It is applicable to general multipartite systems. We show that there are entanglement monotones corresponding to singlet representations of the LU group. They can be evaluated efficiently in an algebraic way, and experimentally measurable by local projective measurements of the copies of the state. Nonsinglet representations are also shown to be useful to classify entanglement. Our method reproduces many well-known measures in a unified way.

  1. Pure state consciousness and its local reduction to neuronal space

    NASA Astrophysics Data System (ADS)

    Duggins, A. J.

    2013-01-01

    The single neuronal state can be represented as a vector in a complex space, spanned by an orthonormal basis of integer spike counts. In this model a scalar element of experience is associated with the instantaneous firing rate of a single sensory neuron over repeated stimulus presentations. Here the model is extended to composite neural systems that are tensor products of single neuronal vector spaces. Depiction of the mental state as a vector on this tensor product space is intended to capture the unity of consciousness. The density operator is introduced as its local reduction to the single neuron level, from which the firing rate can again be derived as the objective correlate of a subjective element. However, the relational structure of perceptual experience only emerges when the non-local mental state is considered. A metric of phenomenal proximity between neuronal elements of experience is proposed, based on the cross-correlation function of neurophysiology, but constrained by the association of theoretical extremes of correlation/anticorrelation in inseparable 2-neuron states with identical and opponent elements respectively.

  2. Self-catalytic conversion of pure quantum states

    NASA Astrophysics Data System (ADS)

    Duarte, Cristhiano; Drumond, Raphael C.; Terra Cunha, Marcelo

    2016-04-01

    Conversion of entangled states under (stochastic) local operations and classical communication ((S)LOCC) admits the phenomenon of catalysis. Here we explore the possibility of a copy of the initial state itself performing as a catalyst, which we call a self-catalytic process. We show explicit examples of self-catalysis. Necessary and sufficient conditions for the phenomenon to take place are discussed. We numerically estimate how frequent it is and we show that increasing the number of copies used as catalyst can increase the probability of conversion, but does not make the process deterministic. By the end we conjecture that under LOCC the probability of finding a self-catalytic reaction does not increase monotonically with the dimensions whereas under SLOCC, it does increase.

  3. Robust state transfer in the quantum spin channel via weak measurement and quantum measurement reversal

    NASA Astrophysics Data System (ADS)

    He, Zhi; Yao, Chunmei; Zou, Jian

    2013-10-01

    Using the weak measurement (WM) and quantum measurement reversal (QMR) approach, robust state transfer and entanglement distribution can be realized in the spin-(1)/(2) Heisenberg chain. We find that the ultrahigh fidelity and long distance of quantum state transfer with certain success probability can be obtained using proper WM and QMR, i.e., the average fidelity of a general pure state from 80% to almost 100%, which is almost size independent. We also find that the distance and quality of entanglement distribution for the Bell state and the general Werner mixed state can be obviously improved by the WM and QMR approach.

  4. Long-lived nuclear spin states far from magnetic equivalence.

    PubMed

    Stevanato, Gabriele; Roy, Soumya Singha; Hill-Cousins, Joe; Kuprov, Ilya; Brown, Lynda J; Brown, Richard C D; Pileio, Giuseppe; Levitt, Malcolm H

    2015-02-28

    Clusters of coupled nuclear spins may form long-lived nuclear spin states, which interact weakly with the environment, compared to ordinary nuclear magnetization. All experimental demonstrations of long-lived states have so far involved spin systems which are close to the condition of magnetic equivalence, in which the network of spin-spin couplings is conserved under all pair exchanges of symmetry-related nuclei. We show that the four-spin system of trans-[2,3-(13)C2]-but-2-enedioate exhibits a long-lived nuclear spin state, even though this spin system is very far from magnetic equivalence. The 4-spin long-lived state is accessed by slightly asymmetric chemical substitutions of the centrosymmetric molecular core. The long-lived state is a consequence of the locally centrosymmetric molecular geometry for the trans isomer, and is absent for the cis isomer. A general group theoretical description of long-lived states is presented. It is shown that the symmetries of coherent and incoherent interactions are both important for the existence of long-lived states. PMID:25633837

  5. Separable operations and local operations with classical communication on triqubit pure states

    NASA Astrophysics Data System (ADS)

    Chen, Yang; Kan, Haibin

    2014-12-01

    Entanglement plays an important role in quantum computation and information. We can only manipulate an entangled quantum state shared among several distant parties by local operations with classical communication (LOCC). Thus, it is of great importance to characterize the conditions by which we can determine whether one pure quantum state can be transformed to another pure state by LOCC. It is well known that separable operations and LOCC are not equivalent. Dozens of results have illustrated this difference. Little do we know about this difference despite these recent results. It is shown in this paper that if the initial state |ψ > and final state |ϕ > are genuine tripartite pure states in the Greenberger-Horne-Zeilinger (GHZ) class then |ψ > can be transformed to |ϕ > by separable operations if and only if |ψ > can be transformed to |ϕ > by deterministic LOCC. That is, SEP equals LOCC on tripartite GHZ states.

  6. Local unitary invariants for N-qubit pure states

    SciTech Connect

    Sharma, S. Shelly; Sharma, N. K.

    2010-11-15

    The concept of negativity font, a basic unit of multipartite entanglement, is introduced. Transformation properties of determinants of negativity fonts under local unitary (LU) transformations are exploited to obtain relevant N-qubit polynomial invariants and construct entanglement monotones from first principles. It is shown that entanglement monotones that detect the entanglement of specific parts of the composite system may be constructed to distinguish between states with distinct types of entanglement. The structural difference between entanglement monotones for an odd and even number of qubits is brought out.

  7. Relation between catalyst-assisted transformation and multiple-copy transformation for bipartite pure states

    SciTech Connect

    Feng Yuan; Duan Runyao; Ying Mingsheng

    2006-10-15

    We show that in some cases, catalyst-assisted entanglement transformation cannot be implemented by multiple-copy transformation for pure states. This fact, together with the result we obtained in R. Y. Duan, Y. Feng, X. Li, and M. S. Ying, Phys. Rev. A 71, 042319 (2005), namely that the latter can be completely implemented by the former, indicates that catalyst-assisted transformation is strictly more powerful than multiple-copy transformation. For the purely probabilistic setting we find, however, these two kinds of transformations are geometrically equivalent in the sense that the sets of pure states that can be converted into a given pure state with maximal probabilities not less than a given value have the same closure, regardless of whether catalyst-assisted transformation or multiple-copy transformation is used.

  8. Remote one-qubit-state control using the pure initial state of a two-qubit sender: Selective-region and eigenvalue creation

    NASA Astrophysics Data System (ADS)

    Bochkin, G. A.; Zenchuk, A. I.

    2015-06-01

    We study the problem of remote one-qubit mixed state creation using a pure initial state of two-qubit sender and spin-1/2 chain as a connecting line. We express the parameters of creatable states in terms of transition amplitudes. We show that the creation of a complete receiver's state space can be achieved only in the chain engineered for the one-qubit perfect state transfer (PST) (for instance, in the fully engineered Ekert chain); the chain can be arbitrarily long in this case. As for the homogeneous chain, the creatable receiver's state region decreases quickly with the chain length. Both homogeneous chains and chains engineered for PST can be used for the purpose of selective state creation, when only the restricted part of the whole receiver's state space is of interest. Among the parameters of the receiver's state, the eigenvalue is the most hard to create and therefore deserves special study. Regarding the homogeneous spin chain, an arbitrary eigenvalue can be created only if the chain is of no more than 34 nodes. The alternating chain allows us to increase this length to up to 68 nodes.

  9. Decontaminating Solar Wind Samples with the Genesis Ultra-Pure Water Megasonic Wafer Spin Cleaner

    NASA Technical Reports Server (NTRS)

    Calaway, Michael J.; Rodriquez, M. C.; Allton, J. H.; Stansbery, E. K.

    2009-01-01

    The Genesis sample return capsule, though broken during the landing impact, contained most of the shattered ultra-pure solar wind collectors comprised of silicon and other semiconductor wafers materials. Post-flight analysis revealed that all wafer fragments were littered with surface particle contamination from spacecraft debris as well as soil from the impact site. This particulate contamination interferes with some analyses of solar wind. In early 2005, the Genesis science team decided to investigate methods for removing the surface particle contamination prior to solar wind analysis.

  10. Geometric characterization of separability and entanglement in pure Gaussian states by single-mode unitary operations

    SciTech Connect

    Adesso, Gerardo; Giampaolo, Salvatore M.; Illuminati, Fabrizio

    2007-10-15

    We present a geometric approach to the characterization of separability and entanglement in pure Gaussian states of an arbitrary number of modes. The analysis is performed adapting to continuous variables a formalism based on single subsystem unitary transformations that has been recently introduced to characterize separability and entanglement in pure states of qubits and qutrits [S. M. Giampaolo and F. Illuminati, Phys. Rev. A 76, 042301 (2007)]. In analogy with the finite-dimensional case, we demonstrate that the 1xM bipartite entanglement of a multimode pure Gaussian state can be quantified by the minimum squared Euclidean distance between the state itself and the set of states obtained by transforming it via suitable local symplectic (unitary) operations. This minimum distance, corresponding to a, uniquely determined, extremal local operation, defines an entanglement monotone equivalent to the entropy of entanglement, and amenable to direct experimental measurement with linear optical schemes.

  11. Geometric characterization of separability and entanglement in pure Gaussian states by single-mode unitary operations

    NASA Astrophysics Data System (ADS)

    Adesso, Gerardo; Giampaolo, Salvatore M.; Illuminati, Fabrizio

    2007-10-01

    We present a geometric approach to the characterization of separability and entanglement in pure Gaussian states of an arbitrary number of modes. The analysis is performed adapting to continuous variables a formalism based on single subsystem unitary transformations that has been recently introduced to characterize separability and entanglement in pure states of qubits and qutrits [S. M. Giampaolo and F. Illuminati, Phys. Rev. A 76, 042301 (2007)]. In analogy with the finite-dimensional case, we demonstrate that the 1×M bipartite entanglement of a multimode pure Gaussian state can be quantified by the minimum squared Euclidean distance between the state itself and the set of states obtained by transforming it via suitable local symplectic (unitary) operations. This minimum distance, corresponding to a , uniquely determined, extremal local operation, defines an entanglement monotone equivalent to the entropy of entanglement, and amenable to direct experimental measurement with linear optical schemes.

  12. Phonon induced pure dephasing process of excitonic state in colloidal semiconductor quantum dots

    NASA Astrophysics Data System (ADS)

    Huang, Tongyun; Han, Peng; Wang, Xinke; Feng, Shengfei; Sun, Wenfeng; Ye, Jiasheng; Zhang, Yan

    2016-04-01

    We present a theoretical study on the pure dephasing process of colloidal semiconductor quantum dots induced by lattice vibrations using continuum model calculations. By solving the time dependent Liouville-von Neumann equation, we present the ultrafast Rabi oscillations between excitonic state and virtual state via exciton-phonon interaction and obtain the pure dephasing time from the fast decayed envelope of the Rabi oscillations. The interaction between exciton and longitudinal optical phonon vibration is found to dominate the pure dephasing process and the dephasing time increases nonlinearly with the reduction of exciton-phonon coupling strength. We further find that the pure dephasing time of large quantum dots is more sensitive to temperature than small quantum dots.

  13. Localized States Influence Spin Transport in Epitaxial Graphene

    NASA Astrophysics Data System (ADS)

    Maassen, T.; van den Berg, J. J.; Huisman, E. H.; Dijkstra, H.; Fromm, F.; Seyller, T.; van Wees, B. J.

    2013-02-01

    We developed a spin transport model for a diffusive channel with coupled localized states that result in an effective increase of spin precession frequencies and a reduction of spin relaxation times in the system. We apply this model to Hanle spin precession measurements obtained on monolayer epitaxial graphene on SiC(0001). Combined with newly performed measurements on quasi-free-standing monolayer epitaxial graphene on SiC(0001) our analysis shows that the different values for the diffusion coefficient measured in charge and spin transport measurements on monolayer epitaxial graphene on SiC(0001) and the high values for the spin relaxation time can be explained by the influence of localized states arising from the buffer layer at the interface between the graphene and the SiC surface.

  14. Entanglement of electronic subbands and coherent superposition of spin states in a Rashba nanoloop

    NASA Astrophysics Data System (ADS)

    Safaiee, R.; Golshan, M. M.

    2011-10-01

    The present work is concerned with an analysis of the entanglement between the electronic coherent superpositions of spin states and subbands in a quasi-one-dimensional Rashba nanoloop acted upon by a strong perpendicular magnetic field. We explicitly include the confining potential and the Rashba spin-orbit coupling into the Hamiltonian and then proceed to calculate the von Neumann entropy, a measure of entanglement, as a function of time. An analysis of the von Neumann entropy demonstrates that, as expected, the dynamics of entanglement strongly depends upon the initial state and electronic subband excitations. When the initial state is a pure one formed by a subband excitation and the z-component of spin states, the entanglement exhibits periodic oscillations with local minima (dips). On the other hand, when the initial state is formed by the subband states and a coherent superposition of spin states, the entanglement still periodically oscillates, exhibiting stronger correlations, along with elimination of the dips. Moreover, in the long run, the entanglement for the latter case undergoes the phenomenon of collapse-revivals. This behaviour is absent for the first case of the initial states. We also show that the degree of entanglement strongly depends upon the electronic subband excitations in both cases.

  15. Knitting distributed cluster-state ladders with spin chains

    SciTech Connect

    Ronke, R.; D'Amico, I.; Spiller, T. P.

    2011-09-15

    Recently there has been much study on the application of spin chains to quantum state transfer and communication. Here we discuss the utilization of spin chains (set up for perfect quantum state transfer) for the knitting of distributed cluster-state structures, between spin qubits repeatedly injected and extracted at the ends of the chain. The cluster states emerge from the natural evolution of the system across different excitation number sectors. We discuss the decohering effects of errors in the injection and extraction process as well as the effects of fabrication and random errors.

  16. Theory of resonance fluorescence from a solid-state cavity QED system: Effects of pure dephasing

    SciTech Connect

    Koshino, Kazuki

    2011-09-15

    We theoretically analyze the resonance fluorescence of a solid-state cavity quantum electrodynamics (QED) system that consists of a quantum dot and a cavity. We clarify the effects of pure dephasing by investigating the elastic and inelastic scattering probabilities, the fluorescence power spectrum, and the energy exchange with the environment. Pure dephasing interactions with the environment both enhance nonresonant coupling between the dot and the cavity and enable the pump light to continuously absorb energy from the environment under appropriate conditions.

  17. Simulating spin-boson models with matrix product states

    NASA Astrophysics Data System (ADS)

    Wall, Michael; Safavi-Naini, Arghavan; Rey, Ana Maria

    2016-05-01

    The global coupling of few-level quantum systems (``spins'') to a discrete set of bosonic modes is a key ingredient for many applications in quantum science, including large-scale entanglement generation, quantum simulation of the dynamics of long-range interacting spin models, and hybrid platforms for force and spin sensing. In many situations, the bosons are integrated out, leading to effective long-range interactions between the spins; however, strong spin-boson coupling invalidates this approach, and spin-boson entanglement degrades the fidelity of quantum simulation of spin models. We present a general numerical method for treating the out-of-equilibrium dynamics of spin-boson systems based on matrix product states. While most efficient for weak coupling or small numbers of boson modes, our method applies for any spatial and operator dependence of the spin-boson coupling. In addition, our approach allows straightforward computation of many quantities of interest, such as the full counting statistics of collective spin measurements and quantum simulation infidelity due to spin-boson entanglement. We apply our method to ongoing trapped ion quantum simulator experiments in analytically intractable regimes. This work is supported by JILA-NSF-PFC-1125844, NSF-PIF- 1211914, ARO, AFOSR, AFOSR-MURI, and the NRC.

  18. Long-lived states with well-defined spins in spin-1 /2 homogeneous Bose gases

    NASA Astrophysics Data System (ADS)

    Yurovsky, Vladimir A.

    2016-02-01

    Many-body eigenfunctions of the total spin operator can be constructed from the spin and spatial wave functions with nontrivial permutation symmetries. Spin-dependent interactions can lead to relaxation of the spin eigenstates to the thermal equilibrium. A mechanism that stabilizes the many-body entangled states is proposed here. Surprisingly, despite coupling with the chaotic motion of the spatial degrees of freedom, the spin relaxations can be suppressed by destructive quantum interference due to spherical vector and tensor terms of the spin-dependent interactions. Tuning the scattering lengths by the method of Feshbach resonances, readily available in cold atomic laboratories, can enhance the relaxation time scales by several orders of magnitude.

  19. Anticoherence of spin states with point-group symmetries

    NASA Astrophysics Data System (ADS)

    Baguette, D.; Damanet, F.; Giraud, O.; Martin, J.

    2015-11-01

    We investigate multiqubit permutation-symmetric states with maximal entropy of entanglement. Such states can be viewed as particular spin states, namely anticoherent spin states. Using the Majorana representation of spin states in terms of points on the unit sphere, we analyze the consequences of a point-group symmetry in their arrangement on the quantum properties of the corresponding state. We focus on the identification of anticoherent states (for which all reduced density matrices in the symmetric subspace are maximally mixed) associated with point-group-symmetric sets of points. We provide three different characterizations of anticoherence and establish a link between point symmetries, anticoherence, and classes of states equivalent through stochastic local operations with classical communication. We then investigate in detail the case of small numbers of qubits and construct infinite families of anticoherent states with point-group symmetry of their Majorana points, showing that anticoherent states do exist to arbitrary order.

  20. Charge-ordering cascade with spin-orbit Mott dimer states in metallic iridium ditelluride.

    PubMed

    Ko, K-T; Lee, H-H; Kim, D-H; Yang, J-J; Cheong, S-W; Eom, M J; Kim, J S; Gammag, R; Kim, K-S; Kim, H-S; Kim, T-H; Yeom, H-W; Koo, T-Y; Kim, H-D; Park, J-H

    2015-01-01

    Spin-orbit coupling results in technologically-crucial phenomena underlying magnetic devices like magnetic memories and energy-efficient motors. In heavy element materials, the strength of spin-orbit coupling becomes large to affect the overall electronic nature and induces novel states such as topological insulators and spin-orbit-integrated Mott states. Here we report an unprecedented charge-ordering cascade in IrTe2 without the loss of metallicity, which involves localized spin-orbit Mott states with diamagnetic Ir(4+)-Ir(4+) dimers. The cascade in cooling, uncompensated in heating, consists of first order-type consecutive transitions from a pure Ir(3+) phase to Ir(3+)-Ir(4+) charge-ordered phases, which originate from Ir 5d to Te 5p charge transfer involving anionic polymeric bond breaking. Considering that the system exhibits superconductivity with suppression of the charge order by doping, analogously to cuprates, these results provide a new electronic paradigm of localized charge-ordered states interacting with itinerant electrons through large spin-orbit coupling. PMID:26059464

  1. Foucault's pendulum, a classical analog for the electron spin state

    NASA Astrophysics Data System (ADS)

    Linck, Rebecca A.

    Spin has long been regarded as a fundamentally quantum phenomena that is incapable of being described classically. To bridge the gap and show that aspects of spin's quantum nature can be described classically, this work uses a classical Lagrangian based on the coupled oscillations of Foucault's pendulum as an analog for the electron spin state in an external magnetic field. With this analog it is possible to demonstrate that Foucault's pendulum not only serves as a basis for explaining geometric phase, but is also a basis for reproducing a broad range of behavior from Zeeman-like frequency splitting to precession of the spin state. By demonstrating that unmeasured electron spin states can be fully described in classical terms, this research opens the door to using the tools of classical physics to examine an inherently quantum phenomenon.

  2. Counterdiabatic driving in spin squeezing and Dicke-state preparation

    NASA Astrophysics Data System (ADS)

    Opatrný, Tomáš; Saberi, Hamed; Brion, Etienne; Mølmer, Klaus

    2016-02-01

    A method is presented to transfer a system of two-level atoms from a spin coherent state to a maximally spin squeezed Dicke state, relevant for quantum metrology and quantum information processing. The initial state is the ground state of an initial linear Hamiltonian that is gradually turned into a final quadratic Hamiltonian whose ground state is the selected Dicke state. We use compensating operators to suppress diabatic transitions to unwanted states that would occur if the change were not slow. We discuss the possibilities of constructing the compensating operators by sequential application of quadratic Hamiltonians available in experiments.

  3. Symmetry and inert states of spin Bose-Einstein condensates

    SciTech Connect

    Yip, S.-K.

    2007-02-15

    We construct the list of all possible inert states of spin Bose-Einstein condensates for S{<=}4. In doing so, we also obtain their symmetry properties. These results are applied to classify line defects of spin condensates in zero magnetic field.

  4. Foucault's Pendulum, Analog for an Electron Spin State

    NASA Astrophysics Data System (ADS)

    Linck, Rebecca

    2012-11-01

    The classical Lagrangian that describes the coupled oscillations of Foucault's pendulum presents an interesting analog to an electron's spin state in an external magnetic field. With a simple modification, this classical Lagrangian yields equations of motion that directly map onto the Schrodinger-Pauli Equation. This analog goes well beyond the geometric phase, reproducing a broad range of behavior from Zeeman-like frequency splitting to precession of the spin state. By demonstrating that unmeasured spin states can be fully described in classical terms, this research opens the door to using the tools of classical physics to examine an inherently quantum phenomenon.

  5. Scalable engineering of multipartite W states in a spin chain

    NASA Astrophysics Data System (ADS)

    Balachandran, Vinitha; Gong, Jiangbin

    2012-06-01

    We propose a scalable scheme for engineering multipartite entangled W states in a Heisenberg spin chain. The rather simple scheme is mainly built on the accumulative angular squeezing technique first proposed in the context of quantum kicked rotor for focusing a rotor to a delta-like angular distribution [I. Sh. Averbukh and R. Arvieu, Phys. Rev. Lett.PRLTAO0031-900710.1103/PhysRevLett.87.163601 87, 163601 (2001)]. We show how the efficient generation of various W states may be achieved by engineering the interaction between a spin chain (short or long) and a time-dependent parabolic magnetic field. Our results may further motivate the use of spin chains as a test bed to investigate complex properties of multipartite entangled states. We further numerically demonstrate that our scheme can be extended to engineer arbitrary spin chain quasimomentum states as well as their superposition states.

  6. Destination state screening of active spaces in spin dynamics simulations

    NASA Astrophysics Data System (ADS)

    Krzystyniak, M.; Edwards, Luke J.; Kuprov, Ilya

    2011-06-01

    We propose a novel avenue for state space reduction in time domain Liouville space spin dynamics simulations, using detectability as a selection criterion - only those states that evolve into or affect other detectable states are kept in the simulation. This basis reduction procedure (referred to as destination state screening) is formally exact and can be applied on top of the existing state space restriction techniques. As demonstrated below, in many cases this results in further reduction of matrix dimension, leading to considerable acceleration of many spin dynamics simulation types. Destination state screening is implemented in the latest version of the Spinach library (http://spindynamics.org).

  7. Spin radical enhanced magnetocapacitance effect in intermolecular excited states.

    PubMed

    Zang, Huidong; Wang, Jianguo; Li, Mingxing; He, Lei; Liu, Zitong; Zhang, Deqing; Hu, Bin

    2013-11-14

    This article reports the magnetocapacitance effect (MFC) based on both pristine polymer MEH-PPV and its composite system doped with spin radicals (6R-BDTSCSB). We observed that a photoexcitation leads to a significant positive MFC in the pristine MEH-PPV. Moreover, we found that a low doping of spin radicals in polymer MEH-PPV causes a significant change on the MFC signal: an amplitude increase and a line-shape narrowing under light illumination at room temperature. However, no MFC signal was observed under dark conditions in either the pristine MEH-PPV or the radical-doped MEH-PPV. Furthermore, the magnitude increase and line-shape narrowing caused by the doped spin radicals are very similar to the phenomena induced by increasing the photoexcitation intensity. Our studies suggest that the MFC is essentially originated from the intermolecular excited states, namely, intermolecular electron-hole pairs, generated by a photoexcitation in the MEH-PPV. More importantly, by comparing the effects of spin radicals and electrically polar molecules on the MFC magnitude and line shape, we concluded that the doped spin radicals can have the spin interaction with intermolecular excited states and consequently affect the internal spin-exchange interaction within intermolecular excited states in the development of MFC. Clearly, our experimental results indicate that dispersing spin radicals forms a convenient method to enhance the magnetocapacitance effect in organic semiconducting materials. PMID:24144347

  8. An Ising spin state explanation for financial asset allocation

    NASA Astrophysics Data System (ADS)

    Horvath, Philip A.; Roos, Kelly R.; Sinha, Amit

    2016-03-01

    We build on the developments in the application of statistical mechanics, notably the identity of the spin degree of freedom in the Ising model, to explain asset price dynamics in financial markets with a representative agent. Specifically, we consider the value of an individual spin to represent the proportional holdings in various assets. We use partial moment arguments to identify asymmetric reactions to information and develop an extension of a plunging and dumping model. This unique identification of the spin is a relaxation of the conventional discrete state limitation on an Ising spin to accommodate a new archetype in Ising model-finance applications wherein spin states may take on continuous values, and may evolve in time continuously, or discretely, depending on the values of the partial moments.

  9. High spin states in {sup 139}Pm

    SciTech Connect

    Dhal, A.; Sinha, R. K.; Chaturvedi, L.; Agarwal, P.; Kumar, S.; Jain, A. K.; Kumar, R.; Govil, I. M.; Mukhopadhyay, S.; Chakraborty, A.; Krishichayan; Ray, S.; Ghugre, S. S.; Sinha, A. K.; Kumar, R.; Singh, R. P.; Muralithar, S.; Bhowmik, R. K.; Pancholi, S. C.; Gupta, J. B.

    2009-07-15

    The odd mass nucleus {sup 139}Pm has been studied to high spins through the {sup 116}Cd({sup 27}Al,4n){sup 139}Pm reaction at an incident beam energy of 120 MeV. The de-exciting {gamma}-rays were detected using an array of 12 Compton suppressed Ge detectors. A total of 46 new levels have been proposed in the present work as a result of the observation of 60 new {gamma}-rays. Four new bands including a {delta}J=1 sequence have been identified and all the earlier reported bands, other than the yrast band, have been extended to higher spins and excitation energy. The spin assignments for most of the newly reported levels have been made using the observed coincidence angular anisotropy. Tilted axis cranking calculations support the interpretation of two of the observed magnetic dipole sequences as examples of magnetic rotational bands.

  10. High-spin states in odd-odd 168Tm

    SciTech Connect

    Cardona, M. A.; Hojman, D.; Davidson, J.; Davidson, M.; Kreiner, A. J.; Bazzacco, D.; Lenzi, S. M.; Rossi Alvarez, C.; Blasi, N.; Debray, M. E.; Levinton, G.; Marti, G.; De Poli, M.; Napoli, D. R.; Lo Bianco, G.

    2007-02-12

    High-spin states in 168Tm were investigated by means of {gamma}-ray spectroscopy techniques using the GASP multidetector array. Rotational bands have been established and identified in terms of their configurations.

  11. Control of Spin States in Triple Quantum Dots

    NASA Astrophysics Data System (ADS)

    Sachrajda, Andrew

    2015-03-01

    A brief review will be given on coherent behaviour in serial triple quantum dots in AlGaAs/GaAs heterostructure related to multi-spin states. One series of experiments involves the application of coherent superpositions of multi-electron states to the transfer of single spins and two-spin states non-locally between edge quantum dots while maintaining the center quantum dot occupation fixed at one or zero electrons. A second series of experiments involves the identification of coherent leakage mechanisms away from targeted encoded three-spin states qubits. Finally, results will be shown which reveal an unexpected control of the gap at the S-T + anticrossing by taking advantage of different nuclear dynamic polarization pumping rates.

  12. Broadband echo sequence using a pi composite pulse for the pure NQR of a spin I = 32 powder sample

    PubMed

    Odin

    2000-04-01

    This work presents a numerical approach to optimizing sequences with composite pulses for the pure NQR of a spin I = 32 powder sample. The calculations are based on a formalism developed in a previous paper, which allows a fast powder-averaging procedure to be implemented. The framework of the Cayley-Klein matrices to describe space rotations by 2 x 2 unitary and unimodular complex matrices is used to calculate the pulse propagators. The object of such a study is to design a high-performance echo sequence composed of a single preparation pulse and a three-pulse composite transfer pulse. We mean a sequence leading to a large excitation bandwidth with a good signal-to-noise ratio, a flat excitation profile near the irradiation frequency, and a good linearity of the phase as a function of frequency offset. Such a composite echo sequence is intended to give a better excitation profile than the classical Hahn (θ)-tau-(2θ) echo sequence. It is argued that in pure NQR of a powder sample, the sequence must be optimized as a whole since both the excitation and the reception of the signal depend on the relative orientation of the crystallites with respect to the coil axis. To our knowledge, this is the first time such a global approach is presented. An extensive numerical study of the composite echo sequence described above is performed in this article. The key of the discrimination between the sequences lies in using the first five reduced moments of the excitation profile as well as an estimator of the phase linearity. Based on such information, we suggest that the echo sequence that best fulfills our criterion is (1)(0)-tau-(0.35)(0)(2.1)(pi)(0.35)(0), the pulse angles omega(RF)t(p) being in radians. The subscripts are the relative pulse phases. We outlined the way to implement the spin echo mapping method to reconstruct large spectra with this sequence, and it is shown that it reduces the acquisition time by a factor of 1.7 if compared to the classical Hahn echo. Some

  13. Quantum metrology with spin cat states under dissipation

    PubMed Central

    Huang, Jiahao; Qin, Xizhou; Zhong, Honghua; Ke, Yongguan; Lee, Chaohong

    2015-01-01

    Quantum metrology aims to yield higher measurement precisions via quantum techniques such as entanglement. It is of great importance for both fundamental sciences and practical technologies, from testing equivalence principle to designing high-precision atomic clocks. However, due to environment effects, highly entangled states become fragile and the achieved precisions may even be worse than the standard quantum limit (SQL). Here we present a high-precision measurement scheme via spin cat states (a kind of non-Gaussian entangled states in superposition of two quasi-orthogonal spin coherent states) under dissipation. In comparison to maximally entangled states, spin cat states with modest entanglement are more robust against losses and their achievable precisions may still beat the SQL. Even if the detector is imperfect, the achieved precisions of the parity measurement are higher than the ones of the population measurement. Our scheme provides a realizable way to achieve high-precision measurements via dissipative quantum systems of Bose atoms. PMID:26647821

  14. Quantum metrology with spin cat states under dissipation.

    PubMed

    Huang, Jiahao; Qin, Xizhou; Zhong, Honghua; Ke, Yongguan; Lee, Chaohong

    2015-01-01

    Quantum metrology aims to yield higher measurement precisions via quantum techniques such as entanglement. It is of great importance for both fundamental sciences and practical technologies, from testing equivalence principle to designing high-precision atomic clocks. However, due to environment effects, highly entangled states become fragile and the achieved precisions may even be worse than the standard quantum limit (SQL). Here we present a high-precision measurement scheme via spin cat states (a kind of non-Gaussian entangled states in superposition of two quasi-orthogonal spin coherent states) under dissipation. In comparison to maximally entangled states, spin cat states with modest entanglement are more robust against losses and their achievable precisions may still beat the SQL. Even if the detector is imperfect, the achieved precisions of the parity measurement are higher than the ones of the population measurement. Our scheme provides a realizable way to achieve high-precision measurements via dissipative quantum systems of Bose atoms. PMID:26647821

  15. Quantum metrology with spin cat states under dissipation

    NASA Astrophysics Data System (ADS)

    Huang, Jiahao; Qin, Xizhou; Zhong, Honghua; Ke, Yongguan; Lee, Chaohong

    2015-12-01

    Quantum metrology aims to yield higher measurement precisions via quantum techniques such as entanglement. It is of great importance for both fundamental sciences and practical technologies, from testing equivalence principle to designing high-precision atomic clocks. However, due to environment effects, highly entangled states become fragile and the achieved precisions may even be worse than the standard quantum limit (SQL). Here we present a high-precision measurement scheme via spin cat states (a kind of non-Gaussian entangled states in superposition of two quasi-orthogonal spin coherent states) under dissipation. In comparison to maximally entangled states, spin cat states with modest entanglement are more robust against losses and their achievable precisions may still beat the SQL. Even if the detector is imperfect, the achieved precisions of the parity measurement are higher than the ones of the population measurement. Our scheme provides a realizable way to achieve high-precision measurements via dissipative quantum systems of Bose atoms.

  16. The equation of state of pure iron-theory and simulation

    NASA Astrophysics Data System (ADS)

    Liu, Haifeng; Wang, Shuaichuang; Zhao, Yanhong; Zhang, Gongmu; Song, Haifeng; Iapcm Team

    2015-06-01

    We calculate the equation of state of pure iron in wide pressure and temperature regime with several models, such as two-body potential, TF and TFC models, and considering electron excite and nucleus anharmonic. In order to address how accuracy of our iron EOS, we simulate EOS by QMD, isentropic compression by fluid dynamic and compare results with expertiment. Our research brings new insights for how to comment the accuracy of equation of state.

  17. Neutrino production states in oscillation phenomena—are they pure or mixed?

    NASA Astrophysics Data System (ADS)

    Ochman, Michał; Szafron, Robert; Zrałek, Marek

    2008-06-01

    General quantum mechanical states of neutrinos produced by mechanisms outside the Standard Model are discussed. The neutrino state is described by the Maki-Nakagawa-Sakata-Pontecorvo unitary mixing matrix only in the case of relativistic neutrinos and Standard Model left-handed charge-current interaction. The problem of Wigner spin rotation caused by Lorentz transformation from the rest production frame to the laboratory frame is considered. Moreover, the mixture of the neutrino states as a function of their energy and parameters from the extension of the Standard Model are investigated. Two sources of mixture, the appearance of subdominant helicity states and mass mixing with several different mixing matrices are studied.

  18. Deterministic LOCC transformation of three-qubit pure states and entanglement transfer

    SciTech Connect

    Tajima, Hiroyasu

    2013-02-15

    A necessary and sufficient condition of the possibility of a deterministic local operations and classical communication (LOCC) transformation of three-qubit pure states is given. The condition shows that the three-qubit pure states are a partially ordered set parametrized by five well-known entanglement parameters and a novel parameter; the five are the concurrences C{sub AB}, C{sub AC}, C{sub BC}, the tangle {tau}{sub ABC} and the fifth parameter J{sub 5} of Acin et al. (2000) Ref. [19], while the other new one is the entanglement charge Q{sub e}. The order of the partially ordered set is defined by the possibility of a deterministic LOCC transformation from a state to another state. In this sense, the present condition is an extension of Nielsen's work (Nielsen (1999) [14]) to three-qubit pure states. We also clarify the rules of transfer and dissipation of the entanglement which is caused by deterministic LOCC transformations. Moreover, the minimum number of times of measurements to reproduce an arbitrary deterministic LOCC transformation between three-qubit pure states is given. - Highlights: Black-Right-Pointing-Pointer We obtained a necessary and sufficient condition for deterministic LOCC of 3 qubits. Black-Right-Pointing-Pointer We clarified rules of entanglement flow caused by measurements. Black-Right-Pointing-Pointer We found a new parameter which is interpreted as 'Charge of Entanglement'. Black-Right-Pointing-Pointer We gave a set of entanglements which determines whether two states are LU-eq. or not. Black-Right-Pointing-Pointer Our approach to deterministic LOCC of 3 qubits may be applicable to N qubits.

  19. Entangled states decoherence in coupled molecular spin clusters

    NASA Astrophysics Data System (ADS)

    Troiani, Filippo; Szallas, Attila; Bellini, Valerio; Affronte, Marco

    2010-03-01

    Localized electron spins in solid-state systems are widely investigated as potential building blocks of quantum devices and computers. While most efforts in the field have been focused on semiconductor low-dimensional structures, molecular antiferromagnets were recently recognized as alternative implementations of effective few-level spin systems. Heterometallic, Cr-based spin rings behave as effective spin-1/2 systems at low temperature and show long decoherence times [1]; besides, they can be chemically linked and magnetically coupled in a controllable fascion [2]. Here, we theoretically investigate the decoherence of the Bell states in such ring dimers, resulting from hyperfine interactions with nuclear spins. Based on a microscopic description of the molecules [3], we simulate the effect of inhomogeneous broadening, spectral diffusion and electron-nuclear entanglement on the electron-spin coherence, estimating the role of the different nuclei (and of possible chemical substitutions), as well as the effect of simple spin-echo sequences. References: [1] F. Troiani, et al., Phys. Rev. Lett. 94, 207208 (2005). [2] G. A. Timco, S: Carretta, F. Troiani et al., Nature Nanotech. 4, 173 (2009). [3] F. Troiani, V. Bellini, and M. Affronte, Phys. Rev. B 77, 054428 (2008).

  20. Separability Criterion for Arbitrary Multipartite Pure State Based on the Rank of Reduced Density Matrix

    NASA Astrophysics Data System (ADS)

    Zhao, Chao; Yang, Guo-wu; Li, Xiao-yu

    2016-09-01

    Nowadays, there are plenty of separability criteria which are used to detect entanglement. Many of them are limited to apply for some cases. In this paper, we propose a separability criterion for arbitrary multipartite pure state which is based on the rank of reduced density matrix. It is proved that the rank of reduced density matrices of a multipartite state is closely related to entanglement. In fact it can be used to characterize entanglement. Our separability criterion is a necessary and sufficient condition for detecting entanglement. Furthermore, it is able to help us find the completely separable form of a multipartite pure state according to some explicit examples. Finally it demonstrates that our method are more suitable for some specific case. Our separability criterion are simple to understand and it is operational.

  1. Separability Criterion for Arbitrary Multipartite Pure State Based on the Rank of Reduced Density Matrix

    NASA Astrophysics Data System (ADS)

    Zhao, Chao; Yang, Guo-wu; Li, Xiao-yu

    2016-04-01

    Nowadays, there are plenty of separability criteria which are used to detect entanglement. Many of them are limited to apply for some cases. In this paper, we propose a separability criterion for arbitrary multipartite pure state which is based on the rank of reduced density matrix. It is proved that the rank of reduced density matrices of a multipartite state is closely related to entanglement. In fact it can be used to characterize entanglement. Our separability criterion is a necessary and sufficient condition for detecting entanglement. Furthermore, it is able to help us find the completely separable form of a multipartite pure state according to some explicit examples. Finally it demonstrates that our method are more suitable for some specific case. Our separability criterion are simple to understand and it is operational.

  2. Open quantum random walks: Bistability on pure states and ballistically induced diffusion

    NASA Astrophysics Data System (ADS)

    Bauer, Michel; Bernard, Denis; Tilloy, Antoine

    2013-12-01

    Open quantum random walks (OQRWs) deal with quantum random motions on a line for systems with internal and orbital degrees of freedom. The internal system behaves as a quantum random gyroscope coding for the direction of the orbital moves. We reveal the existence of a transition, depending on OQRW moduli, in the internal system behaviors from simple oscillations to random flips between two unstable pure states. This induces a transition in the orbital motions from the usual diffusion to ballistically induced diffusion with a large mean free path and large effective diffusion constant at large times. We also show that mixed states of the internal system are converted into random pure states during the process. We touch upon possible experimental realizations.

  3. Mixing nonclassical pure states in a linear-optical network almost always generates modal entanglement

    NASA Astrophysics Data System (ADS)

    Jiang, Zhang; Lang, Mattihas; Caves, Carlton; CenterQuantum Information and Control Collaboration

    2014-03-01

    In quantum optics a pure state is considered classical, relative to the statistics of photodetection, if and only if it is a coherent state. A different and newer notion of nonclassicality is based on modal entanglement. One example that relates these two notions is the Hong-Ou-Mandel effect, where modal entanglement is generated by a beamsplitter from the nonclassical photon-number state | 1 > ⊗ | 1 > . This suggests the beamsplitter or, more generally, linear-optical networks as a mediator of the two notions of nonclassicality. We show the following: Given a nonclassical pure product state input to an N-port linear-optical network, the output is almost always mode entangled; the only exception is a product of squeezed states, all with the same squeezing strength, input to a network that does not mix the squeezed and anti-squeezed quadratures. Our work thus gives a necessary and sufficient condition for a linear network to generate modal entanglement from pure product inputs, a result that is of immediate relevance to the boson sampling problem.

  4. Mixing nonclassical pure states in a linear-optical network almost always generates modal entanglement

    NASA Astrophysics Data System (ADS)

    Jiang, Zhang; Lang, Matthias D.; Caves, Carlton M.

    2013-10-01

    In quantum optics a pure state is considered classical, relative to the statistics of photodetection, if and only if it is a coherent state. A different and newer notion of nonclassicality is based on modal entanglement. One example that relates these two notions is the Hong-Ou-Mandel effect, where modal entanglement is generated by a beamsplitter from the nonclassical photon-number state |1>⊗|1>. This suggests that beamsplitters or, more generally, linear-optical networks are mediators of the two notions of nonclassicality. In this Brief Report, we show the following: Given a nonclassical pure-product-state input to an N-port linear-optical network, the output is almost always mode entangled; the only exception is a product of squeezed states, all with the same squeezing strength, input to a network that does not mix the squeezed and antisqueezed quadratures. Our work thus gives a necessary and sufficient condition for a linear network to generate modal entanglement from pure-product inputs, a result that is of immediate relevance to the boson-sampling problem.

  5. Combustion resistance of the 129Xe hyperpolarized nuclear spin state.

    PubMed

    Stupic, Karl F; Six, Joseph S; Olsen, Michael D; Pavlovskaya, Galina E; Meersmann, Thomas

    2013-01-01

    Using a methane-xenon mixture for spin exchange optical pumping, MRI of combustion was enabled. The (129)Xe hyperpolarized nuclear spin state was found to sufficiently survive the complete passage through the harsh environment of the reaction zone. A velocity profile (V(z)(z)) of a flame was recorded to demonstrate the feasibility of MRI velocimetry of transport processes in combustors. PMID:23165418

  6. Relation between the Greenberger-Horne-Zeilinger-entanglement cost of preparing a multipartite pure state and its quantum discord

    NASA Astrophysics Data System (ADS)

    Yang, Seungho; Jeong, Hyunseok

    2015-08-01

    We investigate how much amount of Greenberger-Horne-Zeilinger (GHZ) entanglement is required in order to prepare a given multipartite state by local operations and classical communication (LOCC). We present a LOCC procedure that asymptotically converts GHZ states into an arbitrary multipartite pure state, whose conversion rate is given by the multipartite discord of the state. This reveals that the GHZ-entanglement cost of preparing a pure state is not higher than the multipartite discord of the state. It also provides an operational interpretation of multipartite discord for pure states, namely, the consumption rate of GHZ entanglement in the devised procedure.

  7. Edge states, spin transport, and impurity-induced local density of states in spin-orbit coupled graphene

    NASA Astrophysics Data System (ADS)

    Seshadri, Ranjani; Sengupta, K.; Sen, Diptiman

    2016-01-01

    We study graphene, which has both spin-orbit coupling (SOC), taken to be of the Kane-Mele form, and a Zeeman field induced due to proximity to a ferromagnetic material. We show that a zigzag interface of graphene having SOC with its pristine counterpart hosts robust chiral edge modes in spite of the gapless nature of the pristine graphene; such modes do not occur for armchair interfaces. Next we study the change in the local density of states (LDOS) due to the presence of an impurity in graphene with SOC and Zeeman field, and demonstrate that the Fourier transform of the LDOS close to the Dirac points can act as a measure of the strength of the spin-orbit coupling; in addition, for a specific distribution of impurity atoms, the LDOS is controlled by a destructive interference effect of graphene electrons which is a direct consequence of their Dirac nature. Finally, we study transport across junctions, which separates spin-orbit coupled graphene with Kane-Mele and Rashba terms from pristine graphene both in the presence and absence of a Zeeman field. We demonstrate that such junctions are generally spin active, namely, they can rotate the spin so that an incident electron that is spin polarized along some direction has a finite probability of being transmitted with the opposite spin. This leads to a finite, electrically controllable, spin current in such graphene junctions. We discuss possible experiments that can probe our theoretical predictions.

  8. Relation Between Stereographic Projection and Concurrence Measure in Bipartite Pure States

    NASA Astrophysics Data System (ADS)

    Najarbashi, G.; Seifi, B.

    2016-06-01

    One-qubit pure states, living on the surface of Bloch sphere, can be mapped onto the usual complex plane by using stereographic projection. In this paper, after reviewing the entanglement of two-qubit pure state, it is shown that the quaternionic stereographic projection is related to concurrence measure. This is due to the fact that every two-qubit state, in ordinary complex field, corresponds to the one-qubit state in quaternionic skew field, called quaterbit. Like the one-qubit states in complex field, the stereographic projection maps every quaterbit onto a quaternion number whose complex and quaternionic parts are related to Schmidt and concurrence terms respectively. Rather, the same relation is established for three-qubit state under octonionic stereographic projection which means that if the state is bi-separable then, quaternionic and octonionic terms vanish. Finally, we generalize recent consequences to 2⊗N and 4⊗N dimensional Hilbert spaces (N ≥ 2) and show that, after stereographic projection, the quaternionic and octonionic terms are entanglement sensitive. These trends are easily confirmed by direct computation for general multi-particle W- and GHZ-states.

  9. DETERMINING TITAN'S SPIN STATE FROM CASSINI RADAR IMAGES

    SciTech Connect

    Stiles, Bryan W.; Hensley, Scott; Ostro, Steven J.; Callahan, Philip S.; Gim, Yonggyu; Hamilton, Gary; Johnson, William T. K.; West, Richard D.; Kirk, Randolph L.; Lee, Ella; Lorenz, Ralph D.; Allison, Michael D.; Iess, Luciano; Del Marmo, Paolo Perci

    2008-05-15

    For some 19 areas of Titan's surface, the Cassini RADAR instrument has obtained synthetic aperture radar (SAR) images during two different flybys. The time interval between flybys varies from several weeks to two years. We have used the apparent misregistration (by 10-30 km) of features between separate flybys to construct a refined model of Titan's spin state, estimating six parameters: north pole right ascension and declination, spin rate, and these quantities' first time derivatives We determine a pole location with right ascension of 39.48 degrees and declination of 83.43 degrees corresponding to a 0.3 degree obliquity. We determine the spin rate to be 22.5781 deg day{sup -1} or 0.001 deg day{sup -1} faster than the synchronous spin rate. Our estimated corrections to the pole and spin rate exceed their corresponding standard errors by factors of 80 and 8, respectively. We also found that the rate of change in the pole right ascension is -30 deg century{sup -1}, ten times faster than right ascension rate of change for the orbit normal. The spin rate is increasing at a rate of 0.05 deg day{sup -1} per century. We observed no significant change in pole declination over the period for which we have data. Applying our pole correction reduces the feature misregistration from tens of km to 3 km. Applying the spin rate and derivative corrections further reduces the misregistration to 1.2 km.

  10. Determining titan's spin state from cassini radar images

    USGS Publications Warehouse

    Stiles, B.W.; Kirk, R.L.; Lorenz, R.D.; Hensley, S.; Lee, E.; Ostro, S.J.; Allison, M.D.; Callahan, P.S.; Gim, Y.; Iess, L.; Del Marmo, P.P.; Hamilton, G.; Johnson, W.T.K.; West, R.D.

    2008-01-01

    For some 19 areas of Titan's surface, the Cassini RADAR instrument has obtained synthetic aperture radar (SAR) images during two different flybys. The time interval between flybys varies from several weeks to two years. We have used the apparent misregistration (by 10-30 km) of features between separate flybys to construct a refined model of Titan's spin state, estimating six parameters: north pole right ascension and declination, spin rate, and these quantities' first time derivatives We determine a pole location with right ascension of 39.48 degrees and declination of 83.43 degrees corresponding to a 0.3 degree obliquity. We determine the spin rate to be 22.5781 deg day -1 or 0.001 deg day-1 faster than the synchronous spin rate. Our estimated corrections to the pole and spin rate exceed their corresponding standard errors by factors of 80 and 8, respectively. We also found that the rate of change in the pole right ascension is -30 deg century-1, ten times faster than right ascension rate of change for the orbit normal. The spin rate is increasing at a rate of 0.05 deg day -1 per century. We observed no significant change in pole declination over the period for which we have data. Applying our pole correction reduces the feature misregistration from tens of km to 3 km. Applying the spin rate and derivative corrections further reduces the misregistration to 1.2 km. ?? 2008. The American Astronomical Society. All rights reserved.

  11. Low-temperature instability of uniform spin precession in the B phase of pure {sup 3}He and {sup 3}He in an aerogel

    SciTech Connect

    Surovtsev, E. V. Fomin, I. A.

    2010-08-15

    The magnetic-field dependences of the threshold temperature of the low-temperature instability of uniform spin precession in pure {sup 3}He-B and {sup 3}He-B in an aerogel have been determined for the bulk mechanism. These dependences appear to be different. The theoretical dependence of the threshold temperature for the pure case has been compared with the experimental dependence. The threshold temperature of the instability for {sup 3}He in the aerogel has been estimated for typical experimental conditions.

  12. Measurements of the spin-orbit interaction and Landé g factor in a pure-phase InAs nanowire double quantum dot in the Pauli spin-blockade regime

    NASA Astrophysics Data System (ADS)

    Wang, Jiyin; Huang, Shaoyun; Lei, Zijin; Pan, Dong; Zhao, Jianhua; Xu, H. Q.

    2016-08-01

    We demonstrate direct measurements of the spin-orbit interaction and Landé g factors in a semiconductor nanowire double quantum dot. The device is made from a single-crystal pure-phase InAs nanowire on top of an array of finger gates on a Si/SiO2 substrate and the measurements are performed in the Pauli spin-blockade regime. It is found that the double quantum dot exhibits a large singlet-triplet energy splitting of ΔST ˜ 2.3 meV, a strong spin-orbit interaction of ΔSO ˜ 140 μeV, and a large and strongly level-dependent Landé g factor of ˜12.5. These results imply that single-crystal pure-phase InAs nanowires are desired semiconductor nanostructures for applications in quantum information technologies.

  13. Investigation of low-spin states in {sup 92}Zr with the (n,n{sup '}{gamma}) reaction

    SciTech Connect

    Fransen, C.; Werner, V.; Jolie, J.; Brentano, P. von; Bandyopadhyay, D.; Boukharouba, N.; Lesher, S.R.; McEllistrem, M.T.; Yates, S.W.; Pietralla, N.

    2005-05-01

    Excited low-spin states of {sup 92}Zr have been studied with the (n,n{sup '}{gamma}) reaction. Comprehensive data on the electromagnetic decay of states with excitation energies up to about 3.8 MeV in particular, lifetimes, {gamma}-ray branching ratios, multipole mixing ratios, and absolute transition strengths have been obtained. The detailed spectroscopic information about the low-spin level scheme enables us to address the predominant proton-neutron symmetry for low-spin states of {sup 92}Zr. These data are compared to those of corresponding states in the N=52 isotone {sup 94}Mo and to a shell model calculation using {sup 88}Sr as an inert core. However, neither a purely collective picture nor the restricted shell model calculation yields a fully satisfactory description of the observed structures.

  14. Observation of a Topological and Parity-Dependent Phase of m=0 Spin States

    SciTech Connect

    Usami, Koji; Kozuma, Mikio

    2007-10-05

    A Ramsey interrogation scheme was used to measure the phase shift of laser-cooled {sup 87}Rb clock-transition pseudospins arising as a result of a reversal of a bias-magnetic field, i.e., B{yields}-B, during the interrogation. While no phase shift occurred when the reversal was sudden, the Ramsey fringes were shifted by a factor of {pi} when the reversal was adiabatic. We thus verified the prediction that the spin states |F,m=0> acquire a purely topological and parity-dependent phase factor of (-1){sup F} as a result of B{yields}-B.

  15. Generation of chiral spin state by quantum simulation

    NASA Astrophysics Data System (ADS)

    Tanamoto, Tetsufumi

    2016-06-01

    Chirality of materials in nature appears when there are asymmetries in their lattice structures or interactions in a certain environment. Recent development of quantum simulation technology has enabled the manipulation of qubits. Accordingly, chirality can be realized intentionally rather than passively observed. Here we theoretically provide simple methods to create a chiral spin state in a spin-1/2 qubit system on a square lattice. First, we show that switching on and off the Heisenberg and X Y interactions produces the chiral interaction directly in the effective Hamiltonian without controlling local fields. Moreover, when initial states of spin qubits are appropriately prepared, we prove that the chirality with desirable phase is dynamically obtained. Finally, even for the case where switching on and off the interactions is infeasible and the interactions are always on, we show that, by preparing an asymmetric initial qubit state, the chirality whose phase is π /2 is dynamically generated.

  16. Matrix product states for su(2) invariant quantum spin chains

    NASA Astrophysics Data System (ADS)

    Zadourian, Rubina; Fledderjohann, Andreas; Klümper, Andreas

    2016-08-01

    A systematic and compact treatment of arbitrary su(2) invariant spin-s quantum chains with nearest-neighbour interactions is presented. The ground-state is derived in terms of matrix product states (MPS). The fundamental MPS calculations consist of taking products of basic tensors of rank 3 and contractions thereof. The algebraic su(2) calculations are carried out completely by making use of Wigner calculus. As an example of application, the spin-1 bilinear-biquadratic quantum chain is investigated. Various physical quantities are calculated with high numerical accuracy of up to 8 digits. We obtain explicit results for the ground-state energy, entanglement entropy, singlet operator correlations and the string order parameter. We find an interesting crossover phenomenon in the correlation lengths.

  17. Improved fair sampling of ground states in Ising spin glasses

    NASA Astrophysics Data System (ADS)

    Katzgraber, Helmut G.; Zhu, Zheng; Ochoa, Andrew J.

    2015-03-01

    Verifying that an optimization approach can sample all solutions that minimize a Hamiltonian is a stringent test for any newly-developed algorithm. While most solvers easily compute the minimum of a cost function for small to moderate input sizes, equiprobable sampling of all ground-state configurations (within Poissonian fluctuations) is much harder to obtain. Most notably, methods such as transverse-field quantum annealing fail in passing this test for certain highly-degenerate problems. Here we present an attempt to sample ground states for Ising spin glasses based on a combination of low-temperature parallel tempering Monte Carlo combined with the cluster algorithm by Houdayer. Because the latter is rejection free and obeys details balance, the ground-state manifold is efficiently sampled. We illustrate the approach for Ising spin glasses on the D-Wave Two quantum annealer topology, known as the Chimera graph, as well as two-dimensional Ising spin glasses.

  18. Stochastic feedback control of quantum transport to realize a dynamical ensemble of two nonorthogonal pure states

    NASA Astrophysics Data System (ADS)

    Daryanoosh, Shakib; Wiseman, Howard M.; Brandes, Tobias

    2016-02-01

    A Markovian open quantum system which relaxes to a unique steady state ρss of finite rank can be decomposed into a finite physically realizable ensemble (PRE) of pure states. That is, as shown by R. I. Karasik and H. M. Wiseman [Phys. Rev. Lett. 106, 020406 (2011), 10.1103/PhysRevLett.106.020406], in principle there is a way to monitor the environment so that in the long-time limit the conditional state jumps between a finite number of possible pure states. In this paper we show how to apply this idea to the dynamics of a double quantum dot arising from the feedback control of quantum transport, as previously considered by C. Pöltl, C. Emary, and T. Brandes [Phys. Rev. B 84, 085302 (2011), 10.1103/PhysRevB.84.085302]. Specifically, we consider the limit where the system can be described as a qubit, and show that while the control scheme can always realize a two-state PRE, in the incoherent-tunneling regime there are infinitely many PREs compatible with the dynamics that cannot be so realized. For the two-state PREs that are realized, we calculate the counting statistics and see a clear distinction between the coherent and incoherent regimes.

  19. Direct measurement of concurrence for atomic two-qubit pure states

    SciTech Connect

    Romero, G.; Lopez, C. E.; Lastra, F.; Retamal, J. C.; Solano, E.

    2007-03-15

    We propose a general scheme to measure the concurrence of an arbitrary two-qubit pure state in atomic systems. The protocol is based on one- and two-qubit operations acting on two available copies of the bipartite system, and followed by a global qubit readout. We show that it is possible to encode the concurrence in the probability of finding all atomic qubits in the ground state. Two possible scenarios are considered: atoms crossing three-dimensional microwave cavities and trapped ion systems.

  20. Manipulating topological states by imprinting non-collinear spin textures

    SciTech Connect

    Streubel, Robert; Han, Luyang; Im, Mi -Young; Kronast, Florian; Rößler, Ulrich K.; Radu, Florin; Abrudan, Radu; Schmidt, Oliver G.; Fischer, Peter; Makarov, Denys

    2015-03-05

    Topological magnetic states, such as chiral skyrmions, are of great scientific interest and show huge potential for novel spintronics applications, provided their topological charges can be fully controlled. So far skyrmionic textures have been observed in noncentrosymmetric crystalline materials with low symmetry and at low temperatures. We propose theoretically and demonstrate experimentally the design of spin textures with topological charge densities that can be tailored at ambient temperatures. Tuning the interlayer coupling in vertically stacked nanopatterned magnetic heterostructures, such as a model system of a Co/Pd multilayer coupled to Permalloy, the in-plane non-collinear spin texture of one layer can be imprinted into the out-of-plane magnetised material. We observe distinct spin textures, e.g. vortices, magnetic swirls with tunable opening angle, donut states and skyrmion core configurations. We show that applying a small magnetic field, a reliable switching between topologically distinct textures can be achieved at remanence

  1. Manipulating topological states by imprinting non-collinear spin textures

    DOE PAGESBeta

    Streubel, Robert; Han, Luyang; Im, Mi -Young; Kronast, Florian; Rößler, Ulrich K.; Radu, Florin; Abrudan, Radu; Lin, Gungun; Schmidt, Oliver G.; Fischer, Peter; et al

    2015-03-05

    Topological magnetic states, such as chiral skyrmions, are of great scientific interest and show huge potential for novel spintronics applications, provided their topological charges can be fully controlled. So far skyrmionic textures have been observed in noncentrosymmetric crystalline materials with low symmetry and at low temperatures. We propose theoretically and demonstrate experimentally the design of spin textures with topological charge densities that can be tailored at ambient temperatures. Tuning the interlayer coupling in vertically stacked nanopatterned magnetic heterostructures, such as a model system of a Co/Pd multilayer coupled to Permalloy, the in-plane non-collinear spin texture of one layer can bemore » imprinted into the out-of-plane magnetised material. We observe distinct spin textures, e.g. vortices, magnetic swirls with tunable opening angle, donut states and skyrmion core configurations. We show that applying a small magnetic field, a reliable switching between topologically distinct textures can be achieved at remanence« less

  2. Relativistic electrons spin states and spin light in dense neutrino fluxes

    NASA Astrophysics Data System (ADS)

    Balantsev, Ilya; Studenikin, Alexander

    2016-05-01

    Relativistic electrons can produce electromagnetic radiation in moving background composed of neutrinos, that is the “spin light of electron in neutrino flux” (SLev ) [1, 2]. In this paper we further specify the electron quantum states in moving neutrino background by introdusing the electron spin operator that enables one to define the electron wave function in an exact and close form. This justifies our previous studies of SLev in dense neutrino fluxes and derivations of the electron energy spectrum, the radiation rate and power, and also the emitted photon energy. We argue that the SLev can have important consequences in different astrophysical settings.

  3. Nuclear states and shapes at high spin. [Good review

    SciTech Connect

    Diamond, R.M.

    1980-08-01

    As angular momentum is added to a nucleus, the balance of forces acting upon it to determine its shape, moment of inertia, mode of rotation, and type of level structure may undergo a series of changes. At relatively low spins a deformed nucleus will rotate collectively, and one may see the effect of Coriolis antipairing in gradually increasing the moment of inertia. Around spin 12 to 16 h-bar there may be an abrupt change (backbending) when a pair of high-j nucleons unpairs and the nucleons align with the axis of rotation; this process allows the nucleus to slow its collective rotation. This process, the start of a sharing of angular momentum between single-particle motion and the collective rotation, gives a lower total energy and corresponds to a change toward triaxiality in the shape of the nucleus. At much higher spins discrete ..gamma..-ray transitions can no longer be observed. This is the regime of continuum spectra; all the information on these high-spin states (to 65 h-bar) is contained in these continuum cascades. Knowledge is accumulating on how to study these spectra, experimentally and theoretically, and new techniques offer promise of revealing a great deal of information about the shapes and properties of very high spin states. 71 references, 34 figures.

  4. Entanglement in bipartite pure states of an interacting boson gas obtained by local projective measurements

    SciTech Connect

    Paraan, Francis N. C.; Korepin, Vladimir E.; Molina-Vilaplana, Javier; Bose, Sougato

    2011-09-15

    We quantify the extractable entanglement of excited states of a Lieb-Liniger gas that are obtained from coarse-grained measurements on the ground state in which the boson number in one of two complementary contiguous partitions of the gas is determined. Numerically exact results obtained from the coordinate Bethe ansatz show that the von Neumann entropy of the resulting bipartite pure state increases monotonically with the strength of repulsive interactions and saturates to the impenetrable-boson limiting value. We also present evidence indicating that the largest amount of entanglement can be extracted from the most probable projected state having half the number of bosons in a given partition. Our study points to a fundamental difference between the nature of the entanglement in free-bosonic and free-fermionic systems, with the entanglement in the former being zero after projection, while that in the latter (corresponding to the impenetrable-boson limit) being nonzero.

  5. Noise resistance of the violation of local causality for pure three-qutrit entangled states

    NASA Astrophysics Data System (ADS)

    Laskowski, Wiesław; Ryu, Junghee; Żukowski, Marek

    2014-10-01

    Bell's theorem started with two qubits (spins 1/2). It is a ‘no-go’ statement on classical (local causal) models of quantum correlations. After 25 years, it turned out that for three qubits the situation is even more astonishing. General statements concerning higher dimensional systems, qutrits, etc, started to appear even later, once the picture with spin (higher than 1/2) was replaced by a broader one, allowing all possible observables. This work is a continuation of the Gdansk effort to take advantage of the fact that Bell's theorem can be put in the form of a linear programming problem, which in turn can be translated into a computer code. Our results are numerical and classify the strength of the violation of local causality by various families of three-qutrit states, as measured by the resistance to noise. This is previously uncharted territory. The results may be helpful in suggesting which three-qutrit states will be handy for applications in quantum information protocols. One of the surprises is that the W state turns out to reveal a stronger violation of local causality than the GHZ (Greenberger-Horne-Zeilinger) state. This article is part of a special issue of Journal of Physics A: Mathematical and Theoretical devoted to ‘50 years of Bell's theorem’.

  6. Hydrogenic states of monopoles in diluted quantum spin ice

    NASA Astrophysics Data System (ADS)

    Petrova, Olga; Moessner, Roderich; Sondhi, S. L.

    2015-09-01

    We consider the effect of adding quantum dynamics to a classical topological spin liquid, with a particular view of how to best detect its presence in experiment. For the Coulomb phase of spin ice, we find quantum effects to be most visible in the gauge-charged monopole excitations. In the presence of weak dilution with nonmagnetic ions we find a particularly crisp phenomenon, namely, the emergence of hydrogenic excited states in which a magnetic monopole is bound to a vacancy at various distances. Via a mapping to an analytically tractable single particle problem on the Bethe lattice, we obtain an approximate expression for the dynamic neutron scattering structure factor.

  7. Enhanced Spin Squeezing in Atomic Ensembles via Control of the Internal Spin States

    NASA Astrophysics Data System (ADS)

    Shojaee, Ezad; Norris, Leigh; Baragiola, Ben; Montano, Enrique; Hemmer, Daniel; Jessen, Poul; Deutsch, Ivan

    2015-05-01

    Abstract: We study the process by which the collective spin squeezing of an ensemble of Cesium atoms is enhanced by control of the internal spin state of the atoms. By increasing the initial atomic projection noise, one can enhance the Faraday interaction that entangles the atoms with a probe. The light acts as a quantum bus for creating atom-atom entanglement via measurement backaction. Further control can be used to transfer this entanglement to metrologically useful squeezing. We numerically simulate this protocol by a stochastic master equation, including QND measurement and optical pumping, which accounts for decoherence and transfer of coherences between magnetic sub-levels. We study the tradeoff between the enhanced entangling interaction and increased rates of decoherence for different initial state preparations. Under realistic conditions, we find that we can achieve squeezing with a ``CAT-State'' superpostion |F = 4, Mz = 4> + |F, Mz = -4> of ~ 9.9 dB and for the spin coherent state |F = 4, Mx = 4> of ~ 7.5 dB. The increased entanglement enabled by the CAT state preparation is partially, but not completely reduced by the increased fragility to decoherence. National Science Foundation.

  8. Photophysical processes of triplet states and radical ions in pure and molecularly doped polymers. Final report

    SciTech Connect

    Burkhart, R.D.

    1998-01-01

    Both the past and current objectives are to learn how to control the rate and direction of triplet exciton migration in both pure and molecularly doped polymer systems. Since triplet excimers are efficient traps for migrating excitons, a secondary objective has been to characterize these excimers with a view toward their use as rate modifiers or excited state quenchers. Further objectives included those stated above as past and current objectives but with an additional goal. The authors learned that fluid solutions of many of the nitrogen containing chromophores with which they work produce both radical cations and anions upon excimer laser excitation. They also learned that a phosphorus analogue behaves similarly. At this time the mechanism of charge generation in these systems is not well established but they do know that the electronically excited states and radical ions can potentially interconvert. They wanted to find out whether or not the pure or molecularly doped polymer systems could be used in a step-wise sequence involving light absorption followed by charge generation. All of their activities are oriented toward the potential end use of polymeric systems in the conversion of light energy to perform various types of useful work.

  9. Flow Injection Potentiometric Assay of Hexoprenaline in Its Pure State, Pharmaceutical Preparations, and Biological Samples

    PubMed Central

    El-Nashar, Rasha M.

    2008-01-01

    Different hexoprenaline (Hx2SO4) conventional and coated wire electrodes were constructed and evaluated. Membranes were based on hexoprenalinium phosphotungstate (Hx-PTA) and hexporenalinium phosphomolybdate (Hx-PMA). The electrodes were fully characterized in terms of their composition, response time, life span, pH, and temperature and then were applied to the potentiometric determination of the hexoprenalinium ion in its pure state, pharmaceutical preparations, and biological samples, urine and plasma, under batch and flow injection conditions. The selectivity of the electrodes towards many inorganic cations, sugars, amino acids, and some other brochodilatures of close chemical composition was also tested. PMID:18483573

  10. Weakly bound states with spin-isospin symmetry

    NASA Astrophysics Data System (ADS)

    Kievsky, A.; Gattobigio, M.

    2016-03-01

    We discuss weakly bound states of a few-fermion system having spin-isospin symmetry. This corresponds to the nuclear physics case in which the singlet, a0, and triplet, a1, n - p scattering lengths are large with respect to the range of the nuclear interaction. The ratio of the two is about a0/a1 ≈ -4.31. This value defines a plane in which a0 and a1 can be varied up to the unitary limit, 1/a0 = 0 and 1/a1 = 0, maintaining its ratio fixed. Using a spin dependant potential model we estimate the three-nucleon binding energy along that plane. This analysis can be considered an extension of the Efimov plot for three bosons to the case of three 1/2-spin-isospin fermions.

  11. Spin-flip scattering and band structure mismatch effect on transport of pure spin across ferromagnetic semimetal/metal material interfaces

    NASA Astrophysics Data System (ADS)

    Pasanai, K.

    2016-03-01

    The tunneling conductance spectra of a ferromagnetic semimetal/metal junction, where there were electrons and holes with the same spin directions as the essential conducting particle, was theoretically studied based on a scattering approach in a ballistic regime. The main area of interest was to perform a high spin polarization by considering the effect of the interfacial scattering at the interface that was composed of normal and spin-flip scattering, the particle effective mass mismatch on the reflection and transmission probabilities, and spin polarization of conductance. It was found that the spin polarization of conductance decreased with increasing spin-flip scattering. Interestingly, the normal scattering can cause the spin polarization of the conductance to reach a maximum value in the presence of both kinds of scattering. When the particle effective mass mismatch was considered, the spin polarization of conductance was large when the electron effective mass in the valence band was smaller than that in the conduction band. However, in this calculation, the results of a ferromagnetic semimetal/metal junction behaved similarly to those of a ferromagnetic metal/metal junction.

  12. High-spin and low-spin mixed state in LaSrCoO4 : An ab initio study

    NASA Astrophysics Data System (ADS)

    Wu, Hua

    2010-03-01

    Spin state is an important issue for many cobaltates, and an intermediate spin (IS) state having a half-filled eg orbital may well be expected for a Co3+ ion in a CoO6 octahedron with a remarkable tetragonal distortion. Here the single-layered perovskite cobaltate LaSrCoO4 , which has a notable tetragonal elongation, is investigated for its spin state and electronic structure, through a set of local-spin-density approximation plus Hubbard U (LSDA+U) calculations including also the multiplet effect and spin-orbit coupling. Counterintuitively, our calculations evidence that the IS state is not the ground state and it would, even if being so, give rise to a wrong ferromagnetic half-metallic solution. We find that a strong band hybridization significantly suppresses a multiplet energy splitting of the IS state. Instead, a high-spin (HS) and low-spin (LS) mixed state turns out to have the lowest total energy among all possibly combined spin states. Moreover, the mixed HS+LS ground state well accounts for the experimental paramagnetic insulating behavior, the effective magnetic moment, and the observed optical spectral features. We also predict that LaSrCoO4 in the mixed HS+LS ground state has a sizeable out-of-plane orbital moment and a local lattice distortion, which would motivate experimental studies.

  13. Direct measurement of the Concurrence of spin-entangled states in a cavity-quantum dot system

    NASA Astrophysics Data System (ADS)

    Dong, Ping; Liu, Jun; Zhang, Li-Hua; Cao, Zhuo-Liang

    2016-08-01

    A scheme for implementing the direct measurement of Concurrence is given in a cavity-quantum dot system. The scenario not only can directly measure the Concurrence of two-spin pure entangled state, but also suitable for the case of mixed state. More importantly, all of the operations are of geometric nature, which depend on the cavity-state-free evolution and can be robust against random operation errors. Our scheme provided an alternative method for directly measuring the degree of entanglement in solid-state system.

  14. Spin-state configuration induced faster spin dynamics in epitaxial La1-xSrxCoO3 thin films

    NASA Astrophysics Data System (ADS)

    Cui, W. Y.; Li, P.; Bai, H. L.

    2015-05-01

    Two important features: spin-state configuration and spin dynamics in phase-separated ferromagnetic/spin-glass epitaxial La1-xSrxCoO3 thin films (x=0.07, 0.17, 0.26, 0.30, 0.40, 0.60) have been investigated and elaborated, proved by both magnetic analyses and first principle calculations. The configuration with high-spin (HS) state Co3+ and low-spin (LS) state Co4+ is considered to be the most stable spin-state configuration for La1-xSrxCoO3 at ground state, which was demonstrated by calculating the magnetic moments of La1-xSrxCoO3, as well as first principle calculation. The stretched Co-O bond by Sr doping causes the decrease of crystal field splitting, resulting in the HS state Co3+ and LS state Co4+. The spin dynamics in the La1-xSrxCoO3 thin films was found to be faster than the classic spin-glass compounds, which is attributed to the higher-spin Co3+, and rather smaller ferromagnetic cluster size (~2.16 to ~21.5 nm) in the epitaxial films than that in referenced polycrystalline compounds (~35 to ~240 nm).

  15. Measurements of the spin states of Europa and Ganymede

    NASA Astrophysics Data System (ADS)

    Margot, Jean-Luc; Padovan, S.; Campbell, D.; Peale, S.; Ghigo, F.

    2013-10-01

    Measuring the spin states of the Galilean satellites holds the key to fundamental interior and surface properties. First, the spin state can reveal the presence of a subsurface ocean: a decoupling between the icy shell and the interior results in a different spin signature than that of a solid body. Second, the value of the obliquity combined with the known gravitational harmonics can provide a direct measurement of the polar moment of inertia, a crucial constraint on interior models. Finally, the obliquity may explain remarkable surface features, such as the distribution and shape of cycloids on Europa, and the direction of strike-slip faults. Here we present the first direct observations of the spin axis orientations of Europa and Ganymede. We use the same Earth-based radar technique that provided measurements of Mercury's obliquity at the sub-arcminute level, observational evidence that the core is molten, and core size estimates [1,2]. The measurements make simultaneous use of the Goldstone Solar System Radar and the Green Bank Telescope located ~3200 km away. It is the correlation of radar echoes received at these two stations that yields superb leverage on the spin state of the illuminated body. Because the Galilean satellites are further away than Mercury, and because they spin faster than Mercury, the signal-to-noise ratio of the observations is reduced by a factor of ~3000. Nevertheless, the telltale correlations are clearly detected in our data. Using measurements at 13 epochs in 2011 and 4 epochs in 2012, we are able to pinpoint Europa's spin axis orientation with a precision of ~0.1 deg, and our result is inconsistent with theoretical or model-based estimates [3,4,5]. For Ganymede, we secured measurements at 3 epochs in 2011 and 2 epochs in 2012, and the larger signal-to-noise ratio results in a comparable precision for the spin axis orientation. References [1] J. L. Margot et al. Science, 316:710, 2007. [2] J. L. Margot et al. JGR (Planets), 117(E16

  16. Electrically tunable spin filtering for electron tunneling between spin-resolved quantum Hall edge states and a quantum dot

    SciTech Connect

    Kiyama, H. Fujita, T.; Teraoka, S.; Oiwa, A.; Tarucha, S.

    2014-06-30

    Spin filtering with electrically tunable efficiency is achieved for electron tunneling between a quantum dot and spin-resolved quantum Hall edge states by locally gating the two-dimensional electron gas (2DEG) leads near the tunnel junction to the dot. The local gating can change the potential gradient in the 2DEG and consequently the edge state separation. We use this technique to electrically control the ratio of the dot–edge state tunnel coupling between opposite spins and finally increase spin filtering efficiency up to 91%, the highest ever reported, by optimizing the local gating.

  17. Probing the spin states of a single acceptor atom.

    PubMed

    van der Heijden, Joost; Salfi, Joe; Mol, Jan A; Verduijn, Jan; Tettamanzi, Giuseppe C; Hamilton, Alex R; Collaert, Nadine; Rogge, Sven

    2014-03-12

    We demonstrate a single-hole transistor using an individual acceptor dopant embedded in a silicon channel. Magneto-transport spectroscopy reveals that the ground state splits as a function of magnetic field into four states, which is unique for a single hole bound to an acceptor in a bulk semiconductor. The two lowest spin states are heavy (|m(j)| = 3/2) and light (|m(j)| = 1/2) hole-like, a two-level system that can be electrically driven and is characterized by a magnetic field dependent and long relaxation time, which are properties of interest for qubits. Although the bulklike spin splitting of a boron atom is preserved in our nanotransistor, the measured Landé g-factors, |g(hh)| = 0.81 ± 0.06 and |g(lh)| = 0.85 ± 0.21 for heavy and light holes respectively, are lower than the bulk value. PMID:24571637

  18. Fractional charge and spin states in topological insulator constrictions

    NASA Astrophysics Data System (ADS)

    Klinovaja, Jelena; Loss, Daniel

    2015-09-01

    We theoretically investigate the properties of two-dimensional topological insulator constrictions both in the integer and fractional regimes. In the presence of a perpendicular magnetic field, the constriction functions as a spin filter with near-perfect efficiency and can be switched by electric fields only. Domain walls between different topological phases can be created in the constriction as an interface between tunneling, magnetic fields, charge density wave, or electron-electron interaction dominated regions. These domain walls host non-Abelian bound states with fractional charge and spin and result in degenerate ground states with parafermions. If a proximity gap is induced bound states give rise to an exotic Josephson current with 8 π periodicity.

  19. Pretty good state transfer of entangled states through quantum spin chains

    NASA Astrophysics Data System (ADS)

    Sousa, Rúben; Omar, Yasser

    2014-12-01

    The XX model with uniform couplings represents the most natural choice for quantum state transfer through spin chains. Given that it has long been established that single-qubit states cannot be transferred with perfect fidelity in this model, the notion of pretty good state transfer has been recently introduced as a relaxation of the constraints on fidelity. In this paper, we study the transfer of multi-qubit entangled and unentangled states through unmodulated spin chains, and we prove that it is possible to have pretty good state transfer of any multi-particle state. This significantly generalizes the previous results on single-qubit state transfer and opens the way to using uniformly coupled spin chains as short-distance quantum channels for the transfer of arbitrary states of any dimension. Our results could be tested with current technology.

  20. Minimum error discrimination for an ensemble of linearly independent pure states

    NASA Astrophysics Data System (ADS)

    Singal, Tanmay; Ghosh, Sibasish

    2016-04-01

    Inspired by the work done by Belavkin (1975 Stochastics 1 315) and independently by Mochon, (2006 Phys. Rev. A 73 032328), we formulate the problem of minimum error discrimination (MED) of any ensemble of n linearly independent pure states by stripping the problem of its rotational covariance and retaining only the rotationally invariant aspect of the problem. This is done by embedding the optimal conditions in a matrix equality as well as matrix inequality. Employing the implicit function theorem in these conditions we get a set of first-order coupled ordinary nonlinear differential equations which can be used to drag the solution from an initial point (where solution is known) to another point (whose solution is sought). This way of obtaining the solution can be done through a simple Taylor series expansion and analytic continuation when required. Thus, we complete the work done by Belavkin and Mochon by ultimately leading their theory to a solution for the MED problem of linearly independent pure state ensembles. We also compare the computational complexity of our technique with the barrier-type interior point method of SDP and show that our technique is computationally as efficient as (actually, a bit more than) the SDP algorithm, with the added advantage of being much simpler to implement.

  1. Evidence for High Spin States in 70Ga

    NASA Astrophysics Data System (ADS)

    Tan, C. L.; Haring-Kaye, R. A.; Jones, K. D.; Le, K. Q.; Döring, J.; Abromeit, B.; Dungan, R.; Lubna, R.; Tabor, S. L.; Tai, P.-L.; Tripathi, V.; Vonmoss, J. M.; Morrow, S. I.

    2015-10-01

    High-spin states in the odd-odd 70Ga nucleus were populated at Florida State University using the 62Ni(14C, αpn) fusion-evaporation reaction at a beam energy of 50 MeV. Gamma rays that depopulated the 70Ga excited states were recorded in coincidence with a Compton-suppressed Ge array consisting of three clover detectors and seven single-crystal detectors. The existing 70Ga level scheme was modified, enhanced, and extended to higher spin with the addition of eight new transitions based on the analysis of double- and triple-coincidence γ-ray spectra. Five of these transitions are associated with a new rotational band that may be based on the occupation of the g9 / 2 orbital by the unpaired proton and neutron. The normalized energy differences between adjacent spin states in this new band indicate a signature-splitting pattern that is characteristic of other such bands in neighboring odd-odd nuclei. Similarly, the kinematic moments of inertia deduced for this decay sequence evolve with angular frequency in a manner typical of analogous bands in other odd-odd nuclei in this mass region.

  2. Exotic Paired States with Anisotropic Spin-Dependent Fermi Surfaces

    SciTech Connect

    Feiguin, Adrian E.; Fisher, Matthew P. A.

    2009-07-10

    We propose a model for realizing exotic paired states in cold Fermi gases by using a spin-dependent optical lattice to engineer mismatched Fermi surfaces for each hyperfine species. The BCS phase diagram shows a stable paired superfluid state with coexisting pockets of momentum space with gapless unpaired carriers, similar to the Sarma state in polarized mixtures, but in our case the system is unpolarized. We propose the possible existence of an exotic 'Cooper-pair Bose-metal' phase, which has a gap for single fermion excitations but gapless and uncondensed 'Cooper-pair' excitations residing on a 'Bose surface' in momentum space.

  3. Maximally entangled set of tripartite qutrit states and pure state separable transformations which are not possible via local operations and classical communication

    NASA Astrophysics Data System (ADS)

    Hebenstreit, M.; Spee, C.; Kraus, B.

    2016-01-01

    Entanglement is the resource to overcome the restriction of operations to local operations assisted by classical communication (LOCC). The maximally entangled set (MES) of states is the minimal set of n -partite pure states with the property that any truly n -partite entangled pure state can be obtained deterministically via LOCC from some state in this set. Hence, this set contains the most useful states for applications. In this work, we characterize the MES for generic three-qutrit states. Moreover, we analyze which generic three-qutrit states are reachable (and convertible) under LOCC transformations. To this end, we study reachability via separable operations (SEP), a class of operations that is strictly larger than LOCC. Interestingly, we identify a family of pure states that can be obtained deterministically via SEP but not via LOCC. This gives an affirmative answer to the question of whether there is a difference between SEP and LOCC for transformations among pure states.

  4. Using corresponding state theory to obtain intermolecular potentials to calculate pure liquid shock Hugoniots

    SciTech Connect

    Hobbs, M.L.

    1997-12-01

    Determination of product species, equations-of-state (EOS) and thermochemical properties of high explosives and pyrotechnics remains a major unsolved problem. Although, empirical EOS models may be calibrated to replicate detonation conditions within experimental variability (5--10%), different states, e.g. expansion, may produce significant discrepancy with data if the basic form of the EOS model is incorrect. A more physically realistic EOS model based on intermolecular potentials, such as the Jacobs Cowperthwaite Zwisler (JCZ3) EOS, is needed to predict detonation states as well as expanded states. Predictive capability for any EOS requires a large species data base composed of a wide variety of elements. Unfortunately, only 20 species have known JCZ3 molecular force constants. Of these 20 species, only 10 have been adequately compared to experimental data such as molecular scattering or shock Hugoniot data. Since data in the strongly repulsive region of the molecular potential is limited, alternative methods must be found to deduce force constants for a larger number of species. The objective of the present study is to determine JCZ3 product species force constants by using a corresponding states theory. Intermolecular potential parameters were obtained for a variety of gas species using a simple corresponding states technique with critical volume and critical temperature. A more complex, four parameter corresponding state method with shape and polarity corrections was also used to obtain intermolecular potential parameters. Both corresponding state methods were used to predict shock Hugoniot data obtained from pure liquids. The simple corresponding state method is shown to give adequate agreement with shock Hugoniot data.

  5. All-optical control of a solid-state spin using coherent dark states.

    PubMed

    Yale, Christopher G; Buckley, Bob B; Christle, David J; Burkard, Guido; Heremans, F Joseph; Bassett, Lee C; Awschalom, David D

    2013-05-01

    The study of individual quantum systems in solids, for use as quantum bits (qubits) and probes of decoherence, requires protocols for their initialization, unitary manipulation, and readout. In many solid-state quantum systems, these operations rely on disparate techniques that can vary widely depending on the particular qubit structure. One such qubit, the nitrogen-vacancy (NV) center spin in diamond, can be initialized and read out through its special spin-selective intersystem crossing, while microwave electron spin resonance techniques provide unitary spin rotations. Instead, we demonstrate an alternative, fully optical approach to these control protocols in an NV center that does not rely on its intersystem crossing. By tuning an NV center to an excited-state spin anticrossing at cryogenic temperatures, we use coherent population trapping and stimulated Raman techniques to realize initialization, readout, and unitary manipulation of a single spin. Each of these techniques can be performed directly along any arbitrarily chosen quantum basis, removing the need for extra control steps to map the spin to and from a preferred basis. Combining these protocols, we perform measurements of the NV center's spin coherence, a demonstration of this full optical control. Consisting solely of optical pulses, these techniques enable control within a smaller footprint and within photonic networks. Likewise, this unified approach obviates the need for both electron spin resonance manipulation and spin addressability through the intersystem crossing. This method could therefore be applied to a wide range of potential solid-state qubits, including those which currently lack a means to be addressed. PMID:23610403

  6. Svetlichny's inequality and genuine tripartite nonlocality in three-qubit pure states

    SciTech Connect

    Ajoy, Ashok; Rungta, Pranaw

    2010-05-15

    The violation of the Svetlichny's inequality (SI) [Phys. Rev. D 35, 3066 (1987)] is sufficient but not necessary for genuine tripartite nonlocal correlations. Here we quantify the relationship between tripartite entanglement and the maximum expectation value of the Svetlichny operator (which is bounded from above by the inequality) for the two inequivalent subclasses of pure three-qubit states: the Greenberger-Horne-Zeilinger (GHZ) class and the W class. We show that the maximum for the GHZ-class states reduces to Mermin's inequality [Phys. Rev. Lett. 65, 1838 (1990)] modulo a constant factor, and although it is a function of the three tangle and the residual concurrence, large numbers of states do not violate the inequality. We further show that by design SI is more suitable as a measure of genuine tripartite nonlocality between the three qubits in the W-class states, and the maximum is a certain function of the bipartite entanglement (the concurrence) of the three reduced states, and only when their sum attains a certain threshold value do they violate the inequality.

  7. Chiral Tunneling of Topological States: Towards the Efficient Generation of Spin Current Using Spin-Momentum Locking

    NASA Astrophysics Data System (ADS)

    Habib, K. M. Masum; Sajjad, Redwan N.; Ghosh, Avik W.

    2015-05-01

    We show that the interplay between chiral tunneling and spin-momentum locking of helical surface states leads to spin amplification and filtering in a 3D topological insulator (TI). Our calculations show that the chiral tunneling across a TI p n junction allows normally incident electrons to transmit, while the rest are reflected with their spins flipped due to spin-momentum locking. The net result is that the spin current is enhanced while the dissipative charge current is simultaneously suppressed, leading to an extremely large, gate-tunable spin-to-charge current ratio (˜20 ) at the reflected end. At the transmitted end, the ratio stays close to 1 and the electrons are completely spin polarized.

  8. Lifetime measurement of high spin states in (75) Kr

    SciTech Connect

    Sheikh, Javid; Trivedi, T.; Maurya, K.; Mehrotra, I.; Palit, R.; Naik, Z.; Jain, H. C.; Negi, D.; Mahanto, G.; Kumar, R.; Singh, R.P.; Muralithar, S.; Pancholi, S.C.; Bhowmik, R.K.; Yang, Y-C; Sun, Y.; Dahl, A.; Raju, M.K.; Appannababu, S.; Kumar, S.; Choudhury, D.; Jain, A. K.

    2010-01-01

    The lifetimes of high spin states of {sup 75}Kr have been determined via {sup 50}Cr ({sup 28}Si, 2pn) {sup 75}Kr reaction in positive parity band using the Doppler-shift attenuation method. The transition quadrupole moments Q deduced from lifetime measurements have been compared with {sup 75}Br. Experimental results obtained from lifetime measurement are interpreted in the framework of projected shell model.

  9. Spin imbalance effect on the Larkin-Ovchinnikov-Fulde-Ferrel state

    SciTech Connect

    Yoshii, Ryosuke; Tsuchiya, Shunji; Marmorini, Giacomo; Nitta, Muneto

    2011-07-01

    We study spin imbalance effects on the Larkin-Ovchinnikov-Fulde-Ferrel (LOFF) state relevant for superconductors under a strong magnetic field and spin polarized ultracold Fermi gas. We obtain the exact solution for the condensates with arbitrary spin imbalance and the fermion spectrum perturbatively in the presence of small spin imbalance. We also obtain fermion zero mode exactly without perturbation theory.

  10. SPIN STATE AND MOMENT OF INERTIA CHARACTERIZATION OF 4179 TOUTATIS

    SciTech Connect

    Takahashi, Yu; Scheeres, D. J.; Busch, Michael W.

    2013-10-01

    The 4.5 km long near-Earth asteroid 4179 Toutatis has made close Earth flybys approximately every four years between 1992 and 2012, and has been observed with high-resolution radar imaging during each approach. Its most recent Earth flyby in 2012 December was observed extensively at the Goldstone and Very Large Array radar telescopes. In this paper, Toutatis' spin state dynamics are estimated from observations of five flybys between 1992 and 2008. Observations were used to fit Toutatis' spin state dynamics in a least-squares sense, with the solar and terrestrial tidal torques incorporated in the dynamical model. The estimated parameters are Toutatis' Euler angles, angular velocity, moments of inertia, and the center-of-mass-center-of-figure offset. The spin state dynamics as well as the uncertainties of the Euler angles and angular velocity of the converged solution are then propagated to 2012 December in order to compare the dynamical model to the most recent Toutatis observations. The same technique of rotational dynamics estimation can be applied to any other tumbling body, given sufficiently accurate observations.

  11. Lifetimes of high-spin states in {sup 162}Yb

    SciTech Connect

    Carpenter, M.P.; Janssens, R.V.F.; Henry, R.G.

    1995-08-01

    A measurement on lifetimes of high-spin states in the yrast and near-yrast rotational bands in {sup 162}Yb was carried out at ATLAS in order to determine the evolution of collectivity as a function of angular momentum using the {sup 126}Te({sup 40}Ar,4n){sup 162}Yb reaction at 170 MeV. Previous lifetime measurements in the {sup 164,166,168}Yb isotopes showed a dramatic decrease in the transition quadrupole moment Q{sub t} with increasing spin. It was suggested that this decrease in Q{sub t} is brought about by the rotationally-induced deoccupation of high-j configurations, mainly i{sub 13/2} neutrons. If this interpretation is correct, the heavier isotopes should have a larger decrease in Q{sub t} than the lighter mass nuclides due to the position of the Fermi surface in the i{sub 13/2} subshell. Indeed, {sup 160}Yb does not show a clear decrease in Q{sub t} at high spin. No high spin lifetime information exists for {sup 162}Yb, thus this experiment fills the gap of measured Q{sub t}`s in the light Yb series. The data is currently being analyzed.

  12. Charge asymmetry and relativistic corrections in pure vibrational states of the HD+ ion

    NASA Astrophysics Data System (ADS)

    Stanke, Monika; Adamowicz, Ludwik

    2014-03-01

    In this work we present very accurate quantum-mechanical calculations of all bound pure vibrational states of the HD+ ion performed without the Born-Oppenheimer (BO) approximation. All three particles forming the system are treated on equal footing. The approach involves separating the center-of-mass motion from the laboratory-frame nonrelativistic Hamiltonian and expending the wave function of each considered state in terms of all-particle explicitly correlated Gaussian functions. The Gaussian exponential parameters are variationally optimized with the aid of the analytical energy gradient calculated with respect to these parameters. For each state the leading relativistic corrections are calculated as expectation values of the corresponding operators with the non-BO wave function of the state. The non-BO approach allows us to directly describe the charge asymmetry in HD+ which is due to the nuclear-mass asymmetry. The effect increases with the vibrational excitation and affects the values of the relativistic corrections. This phenomenon is the focus of the present study.

  13. Perfect inverse spin Hall effect and inverse Edelstein effect due to helical spin-momentum locking in topological surface states

    NASA Astrophysics Data System (ADS)

    Luo, Wei; Deng, W. Y.; Geng, Hao; Chen, M. N.; Shen, R.; Sheng, L.; Xing, D. Y.

    2016-03-01

    We present a theory for the inverse spin Hall effect in a thin film of topological insulator (TI) Bi2Se3 , connected to a reservoir with applied spin bias, in the ballistic regime. In the case that either the spin polarization of the spin bias is along the longitudinal direction, or the hybridization gap Δ of the surface states vanishes, the spin Hall angle Θsh tends to infinity, indicating that the spin bias is perfectly converted into a measurable transverse charge current, essentially without generating a longitudinal spin current in the TI. In other cases, with increasing the Fermi energy EF from the bottom of the conduction band of surface states, Θsh grows continuously from zero and exhibits an interesting linear dependence on EF/Δ for EF≫Δ . We also find that the inverse Edelstein effect occurs, when the in-plane transverse component of the spin polarization vector is nonzero. The spin-to-charge conversion becomes complete, when the spin polarization vector is along the transverse direction, or the hybridization gap Δ vanishes.

  14. π Spin Berry Phase in a Quantum-Spin-Hall-Insulator-Based Interferometer: Evidence for the Helical Spin Texture of the Edge States

    NASA Astrophysics Data System (ADS)

    Chen, Wei; Deng, Wei-Yin; Hou, Jing-Min; Shi, D. N.; Sheng, L.; Xing, D. Y.

    2016-08-01

    The quantum spin Hall insulator is characterized by helical edge states, with the spin polarization of the electron being locked to its direction of motion. Although the edge-state conduction has been observed, unambiguous evidence of the helical spin texture is still lacking. Here, we investigate the coherent edge-state transport in an interference loop pinched by two point contacts. Because of the helical character, the forward interedge scattering enforces a π spin rotation. Two successive processes can only produce a nontrivial 2 π or trivial 0 spin rotation, which can be controlled by the Rashba spin-orbit coupling. The nontrivial spin rotation results in a geometric π Berry phase, which can be detected by a π phase shift of the conductance oscillation relative to the trivial case. Our results provide smoking gun evidence for the helical spin texture of the edge states. Moreover, it also provides the opportunity to all electrically explore the trajectory-dependent spin Berry phase in condensed matter.

  15. π Spin Berry Phase in a Quantum-Spin-Hall-Insulator-Based Interferometer: Evidence for the Helical Spin Texture of the Edge States.

    PubMed

    Chen, Wei; Deng, Wei-Yin; Hou, Jing-Min; Shi, D N; Sheng, L; Xing, D Y

    2016-08-12

    The quantum spin Hall insulator is characterized by helical edge states, with the spin polarization of the electron being locked to its direction of motion. Although the edge-state conduction has been observed, unambiguous evidence of the helical spin texture is still lacking. Here, we investigate the coherent edge-state transport in an interference loop pinched by two point contacts. Because of the helical character, the forward interedge scattering enforces a π spin rotation. Two successive processes can only produce a nontrivial 2π or trivial 0 spin rotation, which can be controlled by the Rashba spin-orbit coupling. The nontrivial spin rotation results in a geometric π Berry phase, which can be detected by a π phase shift of the conductance oscillation relative to the trivial case. Our results provide smoking gun evidence for the helical spin texture of the edge states. Moreover, it also provides the opportunity to all electrically explore the trajectory-dependent spin Berry phase in condensed matter. PMID:27563984

  16. Charge transfer states appear in the π-conjugated pure hydrocarbon molecule on Cu(111)

    NASA Astrophysics Data System (ADS)

    Yonezawa, Keiichirou; Suda, Yosuke; Yanagisawa, Susumu; Hosokai, Takuya; Kato, Kengo; Yamaguchi, Takuma; Yoshida, Hiroyuki; Ueno, Nobuo; Kera, Satoshi

    2016-04-01

    We report on the results of experimental and theoretical studies on the electronic structure of gas-phase diindenoperylene (DIP) and DIP-monolayer (ML) on Cu(111). Vapor-phase ultraviolet photoelectron spectroscopy (UPS) was realized for 11.3 mg of DIP, giving reference orbital energies of isolated DIP, and UPS and inverse photoemission spectroscopy of DIP-ML/graphite were performed to obtain DIP-ML electronic states at a weak interfacial interaction. Furthermore, first-principles calculation clearly demonstrates the interfacial rearrangement. These results provide evidence that the rearrangement of orbital energies, which is realized in HOMO-LUMO and HOMO-HOMO-1 gaps, brings partially occupied LUMO through the surface-induced aromatic stabilization of DIP, a pure hydrocarbon molecule, on Cu(111).

  17. Quantum pump in quantum spin Hall edge states

    NASA Astrophysics Data System (ADS)

    Cheng, Fang

    2016-09-01

    We present a theory for quantum pump in a quantum spin Hall bar with two quantum point contacts (QPCs). The pump currents can be generated by applying harmonically modulating gate voltages at QPCs. The phase difference between the gate voltages introduces an effective gauge field, which breaks the time-reversal symmetry and generates pump currents. The pump currents display very different pump frequency dependence for weak and strong e-e interaction. These unique properties are induced by the helical feature of the edge states, and therefore can be used to detect and control edge state transport.

  18. Lifetimes Measurement for High Spin States in 107Ag

    NASA Astrophysics Data System (ADS)

    Yao, S. H.; Wu, X. G.; He, C. Y.; Zhang, B.; Zheng, Y.; Li, G. S.; Li, C. B.; Hu, S. P.; Cao, X. P.; Yu, B. B.; Zhu, L. H.; Xu, C.; Cheng, Y. Y.

    2013-11-01

    The excited states in 107Ag were populated through the heavy-ion fusion-evaporation reaction 100Mo (11B, 4n) 107Ag at a beam energy of 46 MeV. 12 Compton suppressed HPGe detectors and 2 planar HPGe detectors were employed to detect the de-excited γ rays from the reaction residues. Lifetimes of high spin states in 107Ag have been measured using the Doppler shift attenuation method (DSAM) and the deduced B(M1) and B(E2) transition probabilities have been derived from the measured lifetimes.

  19. Perfect transfer of arbitrary states in quantum spin networks

    SciTech Connect

    Christandl, Matthias; Kay, Alastair; Datta, Nilanjana; Dorlas, Tony C.; Ekert, Artur; Landahl, Andrew J.

    2005-03-01

    We propose a class of qubit networks that admit perfect state transfer of any two-dimensional quantum state in a fixed period of time. We further show that such networks can distribute arbitrary entangled states between two distant parties, and can, by using such systems in parallel, transmit the higher-dimensional systems states across the network. Unlike many other schemes for quantum computation and communication, these networks do not require qubit couplings to be switched on and off. When restricted to N-qubit spin networks of identical qubit couplings, we show that 2 log{sub 3}N is the maximal perfect communication distance for hypercube geometries. Moreover, if one allows fixed but different couplings between the qubits then perfect state transfer can be achieved over arbitrarily long distances in a linear chain. This paper expands and extends the work done by Christandl et al., Phys. Rev. Lett. 92, 187902 (2004)

  20. Muon Spin Rotation Spectroscopy - Utilizing Muons in Solid State Physics

    SciTech Connect

    Suter, Andreas

    2012-10-17

    Over the past decades muon spin rotation techniques (mSR) have established themselves as an invaluable tool to study a variety of static and dynamic phenomena in bulk solid state physics and chemistry. Common to all these approaches is that the muon is utilized as a spin microprobe and/or hydrogen-like probe, implanted in the material under investigation. Recent developments extend the range of application to near surface phenomena, thin film and super-lattice studies. After briefly summarizing the production of so called surface muons used for bulk studies, and discussing the principle differences between pulsed and continuous muon beams, the production of keV-energy muon sources will be discussed. A few topical examples from different active research fields will be presented to demonstrate the power of these techniques.

  1. Computational complexity of nonequilibrium steady states of quantum spin chains

    NASA Astrophysics Data System (ADS)

    Marzolino, Ugo; Prosen, Tomaž

    2016-03-01

    We study nonequilibrium steady states (NESS) of spin chains with boundary Markovian dissipation from the computational complexity point of view. We focus on X X chains whose NESS are matrix product operators, i.e., with coefficients of a tensor operator basis described by transition amplitudes in an auxiliary space. Encoding quantum algorithms in the auxiliary space, we show that estimating expectations of operators, being local in the sense that each acts on disjoint sets of few spins covering all the system, provides the answers of problems at least as hard as, and believed by many computer scientists to be much harder than, those solved by quantum computers. We draw conclusions on the hardness of the above estimations.

  2. Structure and magnetic ground states of spin-orbit coupled compound alpha-RuCl3

    NASA Astrophysics Data System (ADS)

    Banerjee, Arnab; Bridges, Craig; Yan, Jiaqiang; Mandrus, David; Stone, Matthew; Aczel, Adam; Li, Ling; Yiu, Yuen; Lumsden, Mark; Chakoumakos, Bryan; Tennant, Alan; Nagler, Stephen

    2015-03-01

    The layered material alpha-RuCl3 is composed of stacks of weakly coupled honeycomb lattices of octahedrally coordinated Ru3 + ions. The Ru ion ground state has 5 d electrons in the low spin state, with spin-orbit coupling very strong compared to other terms in the single ion Hamiltonian. The material is therefore an excellent candidate for investigating possible Heisenberg-Kitaev physics. In addition, this compound is very amenable to investigation by neutron scattering to explore the magnetic ground state and excitations in detail. In this talk, we discuss the synthesis of phase-pure alpha-RuCl3 and the characterization of the magnetization, susceptibility, and heat-capacity. We also report neutron diffraction on both powder and single crystal alpha-RuCl3, identifying the low temperature magnetic order observed in the material. The results, when compared to theoretical calculations, shed light on the relative importance of Kitaev and Heisenberg terms in the Hamiltonian. The research is supported by the DOE BES Scientific User Facility Division.

  3. Local-spin-density calculations for iron: Effect of spin interpolation on ground-state properties

    NASA Astrophysics Data System (ADS)

    MacLaren, J. M.; Clougherty, D. P.; Albers, R. C.

    1990-08-01

    Scalar-relativistic self-consistent linear muffin-tin orbital (LMTO) calculations for bcc and fcc Fe have been performed with several different local approximations to the exchange and correlation energy density and potential. Overall, in contrast to the conclusions of previous studies, we find that the local-spin-density approximation to exchange and correlation can provide an adequate description of bulk Fe provided that a proper parametrization of the correlation energy density and potential of the homogeneous electron gas over both spin and density is used. Lattice constants, found from the position of the minimum of the total energy as a function of Wigner-Seitz radius, agree to within 1% (for s,p,d LMTO's only) and within 1-2% (for s,p,d,f LMTO's) of the experimental lattice constants for all forms used for the local correlation. The best agreement, however, was obtained using a local correlation potential derived from the Vosko-Wilk-Nusair form for the spin dependence of the correlation energy density. The calculation performed with this correlation potential was also the only calculation to correctly predict a bcc ferromagnetic ground state.

  4. Floquet spin states in graphene under ac-driven spin-orbit interaction

    NASA Astrophysics Data System (ADS)

    López, A.; Sun, Z. Z.; Schliemann, J.

    2012-05-01

    We study the role of periodically driven time-dependent Rashba spin-orbit coupling (RSOC) on a monolayer graphene sample. After recasting the originally 4×4 system of dynamical equations as two time-reversal related two-level problems, the quasienergy spectrum and the related dynamics are investigated via various techniques and approximations. In the static case, the system is gapped at the Dirac point. The rotating wave approximation (RWA) applied to the driven system unphysically preserves this feature, while the Magnus-Floquet approach as well as a numerically exact evaluation of the Floquet equation show that this gap is dynamically closed. In addition, a sizable oscillating pattern of the out-of-plane spin polarization is found in the driven case for states that are completely unpolarized in the static limit. Evaluation of the autocorrelation function shows that the original uniform interference pattern corresponding to time-independent RSOC gets distorted. The resulting structure can be qualitatively explained as a consequence of the transitions induced by the ac driving among the static eigenstates, i.e., these transitions modulate the relative phases that add up to give the quantum revivals of the autocorrelation function. Contrary to the static case, in the driven scenario, quantum revivals (suppressions) are correlated to spin-up (down) phases.

  5. Exchange bias and coercivity for ferromagnets coupled to the domain state and spin glass state

    NASA Astrophysics Data System (ADS)

    Zhan, Xiaozhi; Mao, Zhongquan; Chen, Xi

    2016-05-01

    The exchange bias (EB) effect for systems with a ferromagnetic (FM) layer coupled to bond-diluted pinning layers has been investigated by Monte Carlo simulations. Two bond dilution concentrations are chosen to obtain two kinds of pinning layers: the antiferromagnetic domain state (DS) and the spin glass (SG) state. It is found that when coupled to the more disordered SG state, the ferromagnet shows enhanced EB with higher coercivity due to larger amounts of both frozen and reversible spins at the pinning interface. Spin configurations of the FM/DS interface layer reveal that reversible spins are mostly found in domain boundaries and small domains, while most spins in large domains maintain antiferromagnetic coupling and contribute to the EB effect. The coercivity is linear to the amount of interface reversible spins, but with different slopes in the temperature ranges above or below the blocking temperature t B. This bimodal temperature-dependent coercivity indicates a sudden change in macroscopic interface coupling at the temperature t B.

  6. Approximating the ground state of gapped quantum spin systems

    SciTech Connect

    Michalakis, Spyridon; Hamza, Eman; Nachtergaele, Bruno; Sims, Robert

    2009-01-01

    We consider quantum spin systems defined on finite sets V equipped with a metric. In typical examples, V is a large, but finite subset of Z{sup d}. For finite range Hamiltonians with uniformly bounded interaction terms and a unique, gapped ground state, we demonstrate a locality property of the corresponding ground state projector. In such systems, this ground state projector can be approximated by the product of observables with quantifiable supports. In fact, given any subset {chi} {contained_in} V the ground state projector can be approximated by the product of two projections, one supported on {chi} and one supported on {chi}{sup c}, and a bounded observable supported on a boundary region in such a way that as the boundary region increases, the approximation becomes better. Such an approximation was useful in proving an area law in one dimension, and this result corresponds to a multi-dimensional analogue.

  7. Perfect state transfer over distance-regular spin networks

    SciTech Connect

    Jafarizadeh, M. A.; Sufiani, R.

    2008-02-15

    Christandl et al. have noted that the d-dimensional hypercube can be projected to a linear chain with d+1 sites so that, by considering fixed but different couplings between the qubits assigned to the sites, the perfect state transfer (PST) can be achieved over arbitrarily long distances in the chain [Phys. Rev. Lett. 92, 187902 (2004); Phys. Rev. A 71, 032312 (2005)]. In this work we consider distance-regular graphs as spin networks and note that any such network (not just the hypercube) can be projected to a linear chain and so can allow PST over long distances. We consider some particular spin Hamiltonians which are the extended version of those of Christandl et al. Then, by using techniques such as stratification of distance-regular graphs and spectral analysis methods, we give a procedure for finding a set of coupling constants in the Hamiltonians so that a particular state initially encoded on one site will evolve freely to the opposite site without any dynamical control, i.e., we show how to derive the parameters of the system so that PST can be achieved. It is seen that PST is only allowed in distance-regular spin networks for which, starting from an arbitrary vertex as reference vertex (prepared in the initial state which we wish to transfer), the last stratum of the networks with respect to the reference state contains only one vertex; i.e., stratification of these networks plays an important role which determines in which kinds of networks and between which vertices of them, PST can be allowed. As examples, the cycle network with even number of vertices and d-dimensional hypercube are considered in details and the method is applied for some important distance-regular networks.

  8. Memory effects in Heisenberg spin glasses: Spontaneous restoration of the original spin configuration rather than preservation in a frozen state

    SciTech Connect

    Mamiya, Hiroaki; Nimori, Shigeki

    2012-04-01

    Universality of spin configuration restoration is studied in Heisenberg spin glasses: a dilute magnetic semiconductor Cd{sub 55}Mn{sub 45}Te as well as a dilute magnetic alloy Cu{sub 97}Mn{sub 3}. Reversions of the relaxations of magnetization were observed in both systems undergoing positive/negative temperature cycling under a constant magnetic field. Because the magnetization mirrors evolution of the spin configuration, these reversions indicate that the spin configurations are spontaneously restored to the initially stabilized states when the temperature is returned to the original. Whereas such spin restoration does not occur if the spin glasses are simply frozen, it is possible in the alternative ghost domain scenario of the droplet picture. This finding thus provides fresh insight into the nature of glassy systems.

  9. Self-spin-controlled rotation of spatial states of a Dirac electron in a cylindrical potential via spin orbit interaction

    NASA Astrophysics Data System (ADS)

    Leary, C. C.; Reeb, D.; Raymer, M. G.

    2008-10-01

    Solution of the Dirac equation predicts that when an electron with nonzero orbital angular momentum (OAM) propagates in a cylindrically symmetric potential, its spin and orbital degrees of freedom interact, causing the electron's phase velocity to depend on whether its spin angular momentum (SAM) and OAM vectors are oriented parallel or anti-parallel with respect to each other. This spin-orbit splitting of the electronic dispersion curves can result in a rotation of the electron's spatial state in a manner controlled by the electron's own spin z-component value. These effects persist at non-relativistic velocities. To clarify the physical origin of this effect, we compare solutions of the Dirac equation to perturbative predictions of the Schrödinger-Pauli equation with a spin-orbit term, using the standard Foldy-Wouthuysen Hamiltonian. This clearly shows that the origin of the effect is the familiar relativistic spin-orbit interaction.

  10. Spin State Equilibria of Asteroids due to YORP Effects

    NASA Astrophysics Data System (ADS)

    Golubov, Oleksiy; Scheeres, Daniel J.; Lipatova, Veronika

    2016-05-01

    Spins of small asteroids are controlled by the Yarkovsky--O'Keefe--Radzievskii--Paddack (YORP) effect. The normal version of this effect has two components: the axial component alters the rotation rate, while the obliquity component alters the obliquity. Under this model the rotation state of an asteroid can be described in a phase plane with the rotation rate along the polar radius and the obliquity as the polar angle. The YORP effect induces a phase flow in this plane, which determines the distribution of asteroid rotation rates and obliquities.We study the properties of this phase flow for several typical cases. Some phase flows have stable attractors, while in others all trajectories go to very small or large rotation rates. In the simplest case of zero thermal inertia approximate analytical solutions to dynamics equations are possible. Including thermal inertia and the Tangential YORP effect makes the possible evolutionary scenarios much more diverse. We study possible evolution paths and classify the most general trends. Also we discuss possible implications for the distribution of asteroid rotation rates and obliquities.A special emphasis is put on asteroid (25143) Itokawa, whose shape model is well determined, but who's measured YORP acceleration does not agree with the predictions of normal YORP. We show that Itokawa's rotational state can be explained by the presence of tangential YORP and that it may be in or close to a stable spin state equilibrium. The implications of such states will be discussed.

  11. Habitability of waterworlds: runaway greenhouses, atmospheric expansion, and multiple climate states of pure water atmospheres.

    PubMed

    Goldblatt, Colin

    2015-05-01

    There are four different stable climate states for pure water atmospheres, as might exist on so-called "waterworlds." I map these as a function of solar constant for planets ranging in size from Mars-sized to 10 Earth-mass. The states are as follows: globally ice covered (Ts ⪅ 245 K), cold and damp (270 ⪅ Ts ⪅ 290 K), hot and moist (350 ⪅ Ts ⪅ 550 K), and very hot and dry (Tsx2A86;900 K). No stable climate exists for 290 ⪅ T s ⪅ 350 K or 550 ⪅ Ts ⪅ 900 K. The union of hot moist and cold damp climates describes the liquid water habitable zone, the width and location of which depends on planet mass. At each solar constant, two or three different climate states are stable. This is a consequence of strong nonlinearities in both thermal emission and the net absorption of sunlight. Across the range of planet sizes, I account for the atmospheres expanding to high altitudes as they warm. The emitting and absorbing surfaces (optical depth of unity) move to high altitude, making their area larger than the planet surface, so more thermal radiation is emitted and more sunlight absorbed (the former dominates). The atmospheres of small planets expand more due to weaker gravity; the effective runaway greenhouse threshold is about 35 W m(-2) higher for Mars, 10 W m(-2) higher for Earth or Venus, but only a few W m(-2) higher for a 10 Earth-mass planet. There is an underlying (expansion-neglected) trend of increasing runaway greenhouse threshold with planetary size (40 W m(-2) higher for a 10 Earth-mass planet than for Mars). Summing these opposing trends means that Venus-sized (or slightly smaller) planets are most susceptible to a runaway greenhouse. The habitable zone for pure water atmospheres is very narrow, with an insolation range of 0.07 times the solar constant. A wider habitable zone requires background gas and greenhouse gas: N2 and CO2 on Earth, which are biologically controlled. Thus, habitability depends on inhabitance. PMID:25984919

  12. Habitability of Waterworlds: Runaway Greenhouses, Atmospheric Expansion, and Multiple Climate States of Pure Water Atmospheres

    PubMed Central

    2015-01-01

    Abstract There are four different stable climate states for pure water atmospheres, as might exist on so-called “waterworlds.” I map these as a function of solar constant for planets ranging in size from Mars-sized to 10 Earth-mass. The states are as follows: globally ice covered (Ts⪅245 K), cold and damp (270⪅Ts⪅290 K), hot and moist (350⪅Ts⪅550 K), and very hot and dry (Tsx2A86;900 K). No stable climate exists for 290⪅Ts ⪅350 K or 550⪅Ts⪅900 K. The union of hot moist and cold damp climates describes the liquid water habitable zone, the width and location of which depends on planet mass. At each solar constant, two or three different climate states are stable. This is a consequence of strong nonlinearities in both thermal emission and the net absorption of sunlight. Across the range of planet sizes, I account for the atmospheres expanding to high altitudes as they warm. The emitting and absorbing surfaces (optical depth of unity) move to high altitude, making their area larger than the planet surface, so more thermal radiation is emitted and more sunlight absorbed (the former dominates). The atmospheres of small planets expand more due to weaker gravity; the effective runaway greenhouse threshold is about 35 W m−2 higher for Mars, 10 W m−2 higher for Earth or Venus, but only a few W m−2 higher for a 10 Earth-mass planet. There is an underlying (expansion-neglected) trend of increasing runaway greenhouse threshold with planetary size (40 W m−2 higher for a 10 Earth-mass planet than for Mars). Summing these opposing trends means that Venus-sized (or slightly smaller) planets are most susceptible to a runaway greenhouse. The habitable zone for pure water atmospheres is very narrow, with an insolation range of 0.07 times the solar constant. A wider habitable zone requires background gas and greenhouse gas: N2 and CO2 on Earth, which are biologically controlled. Thus, habitability depends on inhabitance. Key Words

  13. Collectivity of high spin states in {sup 84}Zr

    SciTech Connect

    Lister, C.J.; Blumenthal, D.; Crowell, B.

    1995-08-01

    {sup 84}Zr is one of the most extensively studied of the A {approximately} 80 rotors, both from theoretical and experimental approaches. It was predicted to be a good candidate to support superdeformation, and to show interesting spectroscopic properties including saturation of its shell-model space at lower spin. We performed an experiment using Gammasphere in its early implementation phase. The reaction of {sup 29}Si on {sup 58}Ni was used to strongly populate {sup 84}Zr at high spin. Thin and thick targets were used to allow the extraction of transitional matrix elements at very high spin, and to allow a sensitive search for superdeformed states. Data analysis is in progress. The large data set allowed us to extend the previously known bands considerably. Candidates for a staggered M1-band, found previously {sup 86}Zr, were located. To date, no evidence for superdeformed bands was found. Analysis was slowed by the relocation of all the participants in this experiment, but we hope to complete the lifetime analysis this year. This analysis has become especially topical, due to reported measurements of superdeformation in this region.

  14. Spin-orbit-induced spin-polarized surface states in one-atomic-layer Pb films on Si(111)

    NASA Astrophysics Data System (ADS)

    Lee, Hyungjun; Choi, Hyoung Joon

    2013-03-01

    As a route to spintronics without magnetism, spin-orbit coupling (SOC) generates and manipulates the spin-polarized carriers, thereby providing key ingredients for spin field-effect transistors. Along this line, we investigated the spin-orbit induced effects in Pb monolayers on Si(111) substrates, modeled by √{ 3} ×√{ 3} phase with Pb coverage of 4/3 ML, based on first-principles calculations with the inclusion of SOC. We focus on the electronic structures of surface states with characteristic Rashba-type spin splitting and spin texture as well as the charge flow pattern by calculating the current density distribution for the spin-polarized surface states. We also discuss our results on the difference from the spin splitting in the Shockley surface states on Au(111) surface. This work was supported by the NRF of Korea (Grant No. 2011-0018306), and computational resources have been provided by KISTI Supercomputing Center (Project No. KSC-2012-C2-14).

  15. Measurements of Mercury's spin state and inferences about its interior

    NASA Astrophysics Data System (ADS)

    Margot, J.; Padovan, S.; Peale, S. J.; Solomon, S. C.

    2011-12-01

    Over the past nine years we have used the Green Bank Telescope (GBT) in conjunction with the Goldstone Solar System Radar (GSSR) to characterize the spin state and interior of Mercury. We implemented a technique [1,2] that provides instantaneous spin rate measurements with 10-5 fractional precision and spin orientation measurements at the arcsecond level. On the basis of measurements at 21 distinct epochs between 2002 and 2006, we found observational evidence that Mercury closely follows a Cassini state and that it exhibits forced librations in longitude [3], as predicted by theory [4,5]. A long-period (˜12 year) libration signature may be present in the data. Since 2006 we have secured measurements at 11 additional epochs (out of 23 attempts). We are in the process of re-analyzing the entire set of observations with the goals of (1) refining the determination of the obliquity and of the libration amplitude, two parameters that are critical in the determination of the core size; (2) confirming the presence or absence of a long-period libration component, with the prospect of elucidating the excitation mechanism; (3) quantifying deviations of the pole from the strict Cassini state, which could inform us about dissipation due to solid-body tides and core-mantle interactions. Our first goal is particularly important now that MESSENGER is securing measurements of the low-degree gravitational harmonics with an expected precision of better than 1%. The core-size error budget indicates that the precision of the ground-based estimates of obliquity and librations will ultimately dictate the quality of the core size determination, as well as the attendant inferences regarding the interior structure, thermal evolution, and magnetic field generation of the planet. [1] Green, in Radar Astronomy, McGraw-Hill, 1968. [2] Holin, Radiophys. Quant. Elec. 31, 1988. [3] Margot et al, Science 316, 2007. [4] Peale, Nature 262, 1976. [5] Peale, in Mercury, U. of Arizona Press, 1988.

  16. Quantum error correction for state transfer in noisy spin chains

    NASA Astrophysics Data System (ADS)

    Kay, Alastair

    2016-04-01

    Can robustness against experimental imperfections and noise be embedded into a quantum simulation? In this paper, we report on a special case in which this is possible. A spin chain can be engineered such that, in the absence of imperfections and noise, an unknown quantum state is transported from one end of the chain to the other, due only to the intrinsic dynamics of the system. We show that an encoding into a standard error-correcting code (a Calderbank-Shor-Steane code) can be embedded into this simulation task such that a modified error-correction procedure on readout can recover from sufficiently low rates of noise during transport.

  17. A quantum phase switch between a single solid-state spin and a photon.

    PubMed

    Sun, Shuo; Kim, Hyochul; Solomon, Glenn S; Waks, Edo

    2016-06-01

    Interactions between single spins and photons are essential for quantum networks and distributed quantum computation. Achieving spin-photon interactions in a solid-state device could enable compact chip-integrated quantum circuits operating at gigahertz bandwidths. Many theoretical works have suggested using spins embedded in nanophotonic structures to attain this high-speed interface. These proposals implement a quantum switch where the spin flips the state of the photon and a photon flips the spin state. However, such a switch has not yet been realized using a solid-state spin system. Here, we report an experimental realization of a spin-photon quantum switch using a single solid-state spin embedded in a nanophotonic cavity. We show that the spin state strongly modulates the polarization of a reflected photon, and a single reflected photon coherently rotates the spin state. These strong spin-photon interactions open up a promising direction for solid-state implementations of high-speed quantum networks and on-chip quantum information processors using nanophotonic devices. PMID:26854569

  18. Translation invariant pure state on B = ⊗ j ∈ Z Md ( j ) ( C ) and its split property

    NASA Astrophysics Data System (ADS)

    Mohari, Anilesh

    2015-06-01

    In this paper, we prove that a real lattice symmetric reflection positive translation-invariant pure state of B = ⊗ j ∈ Z Md ( j ) ( C ) admits split property, if and only if its two-point spatial correlation functions decay exponentially. We use amalgamated representation of Cuntz algebras to represent two-point spatial correlation functions on an augmented Hilbert space. The underling symmetries and reflection positive property of the pure state make it possible to investigate its split and decaying two-point correlation functions properties as spectral properties of a contractive self-adjoint operator on the augmented Hilbert space. Haag duality property of the pure state is crucially used in the analysis.

  19. Bistability and steady-state spin squeezing in diamond nanostructures controlled by a nanomechanical resonator

    NASA Astrophysics Data System (ADS)

    Ma, Yong-Hong; Zhang, Xue-Feng; Song, Jie; Wu, E.

    2016-06-01

    As the quantum states of nitrogen vacancy (NV) center can be coherently manipulated and obtained at room temperature, it is important to generate steady-state spin squeezing in spin qubits associated with NV impurities in diamond. With this task we consider a new type of a hybrid magneto-nano-electromechanical resonator, the functionality of which is based on a magnetic-field induced deflection of an appropriate cantilever that oscillates between NV spins in diamond. We show that there is bistability and spin squeezing state due to the presence of the microwave field, despite the damping from mechanical damping. Moreover, we find that bistability and spin squeezing can be controlled by the microwave field and the parameter Vz. Our scheme may have the potential application on spin clocks, magnetometers, and other measurements based on spin-spin system in diamond nanostructures.

  20. Time-Domain Pure-state Polarization Analysis of Surface Waves Traversing California

    SciTech Connect

    Zhang, J; Walter, W R; Lay, T; Wu, R

    2003-11-04

    A time-domain pure-state polarization analysis method is used to characterize surface waves traversing California parallel to the plate boundary. The method is applied to data recorded at four broadband stations in California from twenty-six large, shallow earthquakes which occurred since 1988, yielding polarization parameters such as the ellipticity, Euler angles, instantaneous periods, and wave incident azimuths. The earthquakes are located along the circum-Pacific margin and the ray paths cluster into two groups, with great-circle paths connecting stations MHC and PAS or CMB and GSC. The first path (MHC-PAS) is in the vicinity of the San Andreas Fault System (SAFS), and the second (CMB-GSC) traverses the Sierra Nevada Batholith parallel to and east of the SAFS. Both Rayleigh and Love wave data show refractions due to lateral velocity heterogeneities under the path, indicating that accurate phase velocity and attenuation analysis requires array measurements. The Rayleigh waves are strongly affected by low velocity anomalies beneath Central California, with ray paths bending eastward as waves travel toward the south, while Love waves are less affected, providing observables to constrain the depth extent of the anomalies. Strong lateral gradients in the lithospheric structure between the continent and the ocean are the likely cause of the path deflections.

  1. Thermal Equilibrium of a Macroscopic Quantum System in a Pure State

    NASA Astrophysics Data System (ADS)

    Goldstein, Sheldon; Huse, David A.; Lebowitz, Joel L.; Tumulka, Roderich

    2015-09-01

    We consider the notion of thermal equilibrium for an individual closed macroscopic quantum system in a pure state, i.e., described by a wave function. The macroscopic properties in thermal equilibrium of such a system, determined by its wave function, must be the same as those obtained from thermodynamics, e.g., spatial uniformity of temperature and chemical potential. When this is true we say that the system is in macroscopic thermal equilibrium (MATE). Such a system may, however, not be in microscopic thermal equilibrium (MITE). The latter requires that the reduced density matrices of small subsystems be close to those obtained from the microcanonical, equivalently the canonical, ensemble for the whole system. The distinction between MITE and MATE is particularly relevant for systems with many-body localization for which the energy eigenfuctions fail to be in MITE while necessarily most of them, but not all, are in MATE. We note, however, that for generic macroscopic systems, including those with MBL, most wave functions in an energy shell are in both MATE and MITE. For a classical macroscopic system, MATE holds for most phase points on the energy surface, but MITE fails to hold for any phase point.

  2. Theoretical Study of Renewable Ionic Liquids in the Pure State and with Graphene and Carbon Nanotubes.

    PubMed

    García, Gregorio; Atilhan, Mert; Aparicio, Santiago

    2015-09-17

    The N-ethyl-N-(furan-2-ylmethyl)ethanaminium dihydrogen phosphate ionic liquid was studied as a model of ionic liquids which can be produced from totally renewable sources. A computational study using both molecular dynamics and density functional theory methods was carried out. The properties, structuring, and intermolecular interactions (hydrogen bonding) of this fluid in the pure state were studied as a function of pressure and temperature. Likewise, the adsorption on graphene and the confinement between graphene sheets was also studied. The solvation of single walled carbon nanotubes in the selected ionic liquid was analyzed together with the behavior of ions confined inside these nanotubes. The reported results show remarkable properties for this fluid, which show that many of the most relevant properties of ionic liquids and their ability to interact with carbon nanosystems may be maintained and even improved using new families of renewable compounds instead of classic types of ionic liquids with worse environmental, toxicological, and economical profiles. PMID:26305599

  3. Numerical Modeling of the Central Spin Problem Using the Spin-Coherent-State P Representation

    SciTech Connect

    Al Hassanieh, Khaled A; Dobrovitski, V. V.; Dagotto, Elbio R; Harmon, B. N.

    2006-01-01

    In this work, we consider decoherence of a central spin by a spin bath. In order to study the nonperturbative decoherence regimes, we develop an efficient mean-field-based method for modeling the spin-bath decoherence, based on the P representation of the central spin density matrix. The method can be applied to longitudinal and transverse relaxation at different external fields. In particular, by modeling large-size quantum systems (up to 16 000 bath spins), we make controlled predictions for the slow long-time decoherence of the central spin.

  4. Pure water injection into porous rock with superheated steam and salt in a solid state

    NASA Astrophysics Data System (ADS)

    Montegrossi, G.; Tsypkin, G.; Calore, C.

    2012-04-01

    Most of geothermal fields require injection of fluid into the hot rock to maintain pressure and productivity. The presence of solid salt in porous space may cause an unexpected change in the characteristics of the reservoir and produced fluids, and dramatically affect the profitability of the project. We consider an injection problem of pure water into high temperature geothermal reservoir, saturated with superheated vapour and solid salt. Pure water moves away from injection point and dissolves solid salt. When salty water reaches the low-pressure hot domain, water evaporation occurs and, consequently, salt precipitates. We develop a simplified analytical model of the process and derive the similarity solutions for a 1-D semi-infinite reservoir. These solutions are multi-valued and describe the reduction in permeability and porosity due to salt precipitation at the leading boiling front. If the parameters of the system exceed critical values, then similarity solution ceases to exist. We identify this mathematical behaviour with reservoir sealing in the physical system. The TOUGH2-EWASG code has been used to verify this hypothesis and investigate the precipitate formation for an idealized bounded 1-D geothermal system of a length of 500 m with water injection at one extreme and fluid extraction at the other one. Both boundaries are kept at constant pressure and temperature. The result for the semi-infinite numerical model show that the monotonic grow of the solid salt saturation to reach asymptotic similarity solution generally occurs over a very large length starting from the injection point. Reservoir sealing occurs if solid salt at the initial state occupies a considerable part of the porous space. Numerical experiments for the bounded 500 m system demonstrate that a small amount of salt is enough to get reservoir sealing. Generally, salt tend to accumulate near the production well, and salt plug forms at the elements adjacent to the extraction point. This type

  5. Correlations between metal spin states and vibrational spectra of a trinuclear Fe(II) complex exhibiting spin crossover

    NASA Astrophysics Data System (ADS)

    Gerasimova, Tatiana P.; Katsyuba, Sergey A.; Lavrenova, Ludmila G.; Pelmenschikov, Vladimir; Kaupp, Martin

    2015-12-01

    Combined IR spectroscopic/quantum-chemical analysis of a 4-propyl-1,2,4-triazole trinuclear Fe(II) complex capable of reversible thermal spin crossover has revealed mid-IR bands of the ligand sensitive to the Fe(II) spin state. The character of the correlations found between the intensity and peak position of the triazole bands and the spin state of the metal center depends neither on the identity of the metal nor on the nuclearity of the complex. The found spectral correlations therefore allow analysis of various similar complexes. This is illustrated by the example of experimental IR spectra reported earlier for Fe(II), Co(II), Ni(II), Cu(II) and Zn(II) complexes with triazole ligands. Quantum-chemical IR spectral simulations further suggest that certain ligand bands vary between the states with the same total molecular spin, but different distribution of the spin density between the metal centers. However these variations are too subtle to discriminate between the spin transitions of the central and peripheral Fe(II) ions. The experimentally revealed mid-IR markers are therefore conclusive only for the total molecular spin.

  6. Natural reference for nuclear high-spin states

    SciTech Connect

    Rowley, Neil; Ollier, James; Simpson, John

    2009-08-15

    We suggest two new representations of the data on rotational nuclei. The first is reference-free and the second arises from a natural reference related to the variable moment of inertia model parameters of the ground-state band of the system. As such, neither representation contains any free parameters. By defining a 'configuration spin' we show how a new ground-state band reference can be applied. Its use allows a complete description of the changes associated with the first, and higher, band crossings. We apply these new representations to discuss the nature of the first band crossing along even-even isotopic chains in the erbium and osmium isotopes and to odd-even nuclei in the vicinity of {sup 158}Er.

  7. Investigation of High-Spin States in ^203Rn

    NASA Astrophysics Data System (ADS)

    Beausang, C. W.; Novak, J. R.; Caprio, M.; Casten, R. F.; Cederkall, J.; Cooper, J. R.; Krücken, R.; Wang, Z.; Zamfir, N. V.; Barton, C. J.

    1999-10-01

    High-spin states in ^203Rn were populated following the reaction ^34S + ^174Yb + 5n at beam energies ranging from 160 to 170 MeV. Gamma-rays were detected using the multi-Ge detector array YRAST Ball located at the Wright Nuclear Structure Laboratory. In addition the SCARY array, an array of 28 solar cell detectors, each 1 cm by 1 cm, was arranged around the target at backward angles. These were used to detect fission fragments and hence discriminate against the very large fission background encountered in this reaction. Following our excitation function measurement several transitions can be assigned to ^203Rn, where previously no information was available on excited states. Data analysis is continuing and preliminary results will be presented. This work is supported by the US-DOE under grant number DE-FG02-91ER-40609.

  8. Normal-Deformed High-Spin States in ^81Sr

    NASA Astrophysics Data System (ADS)

    Birriel, I.; Winchell, D. F.; Saladin, J. X.; Cristancho, F.; Landulfo, E.; Wood, V. Q.; Baktash, C.; Brinkman, M. J.; Gross, C. J.; Jin, H.-Q.; Rudolph, D.; Stracener, D. W.; Yu, C.-H.; Devlin, M.; Hua, P.-F.; Korolija, M.; Lafosse, D. R.; Lerma, F.; Sarantites, D. G.; Döring, J.; Sylvan, G.; Tabor, S.; Cederwall, B.; Clark, R. M.; Fallon, P.; Lee, I. Y.; Macchiavelli, A. O.; Maier, M. R.; Rathbun, W.; Vander Mollen, A.; Werner, T. R.

    1998-04-01

    Normal-deformed high-spin states in ^81Sr were populated with the reactions ^58Ni(^29Si,α2p) and ^58Ni(^28Si,4p) with beam energies of 128 and 130 MeV, respectively, from the 88-inch cyclotron at LBNL. Gamma rays from the reactions were detected with Gammasphere, and evaporated α particles and protons were detected with Microball. Our results are consistent with previous work (D.H. Smalley et al, Nucl. Phys. A611 (1996) 96). In addition, two new negative parity rotational bands (built on a 295-241 keV cascade(S.E. Arnell et al, J.Phys. G9, (1983) 1217)) and 11 new side bands have been found. In all, the level scheme has been extended by 65 new states, along with 78 new transitions. The results will be discussed in the framework of the cranked shell model.

  9. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    DOE PAGESBeta

    Jiang, Zilong; Chang, Cui -Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-05-04

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1–x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1–x)2Te3 into a bulk insulator, amore » large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. Lastly, the enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.« less

  10. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states.

    PubMed

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S; MacDonald, Allan H; Shi, Jing

    2016-01-01

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1-x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1-x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics. PMID:27142594

  11. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    NASA Astrophysics Data System (ADS)

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-05-01

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1-x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1-x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.

  12. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    PubMed Central

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-01-01

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1−x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1−x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics. PMID:27142594

  13. Using arterial spin labeling to examine mood states in youth

    PubMed Central

    Mikita, Nina; Mehta, Mitul A; Zelaya, Fernando O; Stringaris, Argyris

    2015-01-01

    Introduction Little is known about the neural correlates of mood states and the specific physiological changes associated with their valence and duration, especially in young people. Arterial spin labeling (ASL) imaging is particularly well-suited to study sustained cerebral states in young people, due to its robustness to low-frequency drift, excellent interscan reliability, and noninvasiveness. Yet, it has so far been underutilized for understanding the neural mechanisms underlying mood states in youth. Methods In this exploratory study, 21 healthy adolescents aged 16 to 18 took part in a mood induction experiment. Neutral, sad, and happy mood states were induced using film clips and explicit instructions. An ASL scan was obtained following presentation of each film clip. Results Mood induction led to robust changes in self-reported mood ratings. Compared to neutral, sad mood was associated with increased regional cerebral blood flow (rCBF) in the left middle frontal gyrus and anterior prefrontal cortex, and decreased rCBF in the right middle frontal gyrus and the inferior parietal lobule. A decrease in self-reported mood from neutral to sad condition was associated with increased rCBF in the precuneus. Happy mood was associated with increased rCBF in medial frontal and cingulate gyri, the subgenual anterior cingulate cortex, and ventral striatum, and decreased rCBF in the inferior parietal lobule. The level of current self-reported depressive symptoms was negatively associated with rCBF change in the cerebellum and lingual gyrus following both sad and happy mood inductions. Conclusions Arterial spin labeling is sensitive to experimentally induced mood changes in healthy young people. The effects of happy mood on rCBF patterns were generally stronger than the effects of sad mood. PMID:26085964

  14. Spin-singlet quantum Hall states and Jack polynomials with a prescribed symmetry

    NASA Astrophysics Data System (ADS)

    Estienne, Benoit; Bernevig, B. Andrei

    2012-04-01

    We show that a large class of bosonic spin-singlet Fractional Quantum Hall model wavefunctions and their quasihole excitations can be written in terms of Jack polynomials with a prescribed symmetry. Our approach describes new spin-singlet quantum Hall states at filling fraction ν=2k/2r-1 and generalizes the (k,r) spin-polarized Jack polynomial states. The NASS and Halperin spin-singlet states emerge as specific cases of our construction. The polynomials express many-body states which contain configurations obtained from a root partition through a generalized squeezing procedure involving spin and orbital degrees of freedom. The corresponding generalized Pauli principle for root partitions is obtained, allowing for counting of the quasihole states. We also extract the central charge and quasihole scaling dimension, and propose a conjecture for the underlying CFT of the (k,r) spin-singlet Jack states.

  15. High-field, hyperpolarized Xe-129 NMR: Preparation and transfer of pure spin-polarized xenon gas to the sample.

    NASA Astrophysics Data System (ADS)

    Patton, B.; Sachs, D. B.; Kuzma, N. N.; Lisitza, N. V.; Happer, W.

    2003-03-01

    Hyperpolarized ^129Xe has already found extensive applications in magnetic resonance imaging(M. S. Albert et al., Nature 370, 199 (1994)) and nuclear magnetic resonance spectroscopy(J. P. Mugler, et al., Magn. Reson. Med. 37, 809 (1997)). Using hyperpolarized xenon in high-field NMR spectroscopy opens up new prospects for medical diagnostics of many pathologies and disorders(R. K. Mazitov, et al., Doklady Biophysics 364-366, 28-31 (1999)). Here we present a new set-up for production(N. N. Kuzma, et al., Phys. Rev. Lett. 88, 147602 (2002)), delivery, and temporary storage of pure hyperpolarized xenon gas for high-field (9.4T) NMR spectroscopy, with an emphasis on in-situ monitoring of ^129Xe polarization along the gas flow path and using a 1.1 T permanent magnet for cryogenic separation of hyperpolarized xenon from the buffer gases.

  16. Molecular Spin Crossover in Slow Motion: Light-Induced Spin-State Transitions in Trigonal Prismatic Iron(II) Complexes.

    PubMed

    Stock, Philipp; Deck, Eva; Hohnstein, Silvia; Korzekwa, Jana; Meyer, Karsten; Heinemann, Frank W; Breher, Frank; Hörner, Gerald

    2016-06-01

    A straightforward access is provided to iron(II) complexes showing exceedingly slow spin-state interconversion by utilizing trigonal-prismatic directing ligands (L(n)) of the extended-tripod type. A detailed analysis of the interrelations between complex structure (X-ray diffraction, density functional theory) and electronic character (SQUID magnetometry, Mössbauer spectroscopy, UV/vis spectroscopy) of the iron(II) center in mononuclear complexes [FeL(n)] reveals spin crossover to occur along a coupled breathing/torsion reaction coordinate, shuttling the complex between the octahedral low-spin state and the trigonal-prismatic high-spin state along Bailar's trigonal twist pathway. We associate both the long spin-state lifetimes in the millisecond domain close to room temperature and the substantial barriers against thermal scrambling (Ea ≈ 33 kJ mol(-1), from Arrhenius analysis) with stereochemical constraints. In particular, the topology of the κ(6)N ligands controls the temporary and structural dynamics during spin crossover. PMID:27159332

  17. Geophysics of Titan from gravity, topography and spin state

    NASA Astrophysics Data System (ADS)

    Nimmo, F.; Bills, B. G.

    2011-12-01

    For the terrestrial planets, combined analyses of gravity and topography have greatly improved our understanding of these bodies' interiors [1]. The spin state and orientation of a planetary body can also be diagnostic of its internal structure [2]. Recently acquired topography [3], gravity [4] and spin pole constraints [5] now permit these kinds of geophysical analyses at Titan. Titan's degree-two gravity coefficients, but not those of its topography, are in the 10/3 ratio expected for a hydrostatic body. One explanation for this discrepancy is the existence of a floating isostatic ice shell whose thickness varies spatially due to tidal dissipation [6]. Shell thickness variations can result in slow non-synchronous rotation [7]. Furthermore, such variations will affect the gravity, an effect that should be taken into account when using gravity to calculate Titan's moment of inertia [4]. The relationship between the degree-three gravity and topography can be used to place constraints on the thickness and rigidity of the ice shell. Based on the inferred heat fluxes of [6], Titan's ice shell is unlikely to be less than 90% compensated at degree three. The measured degree-three gravity [4] and topography [3] coefficients show a strong correlation (r=0.84). For a completely compensated ice shell, the implied shell thickness is about 350 km, while if the shell is 90% compensated the thickness is 250 km. These shell thickness estimates significantly exceed those based on theoretical models [8,9] and surface topography [6]. One possible explanation for this discrepancy is that there are other sources of degree-three gravity (e.g. bumps on the presumed silicate core) that do not contribute significantly to the surface topography. Further gravity observations will help to resolve this issue. If a satellite's spin and orbit poles remain coplanar as the latter precesses around the invariable pole, the satellite is said to occupy a damped Cassini state and the obliquity (angle

  18. Reversible Photoswitching of a Spin-Crossover Molecular Complex in the Solid State at Room Temperature.

    PubMed

    Rösner, Benedikt; Milek, Magdalena; Witt, Alexander; Gobaut, Benoît; Torelli, Piero; Fink, Rainer H; Khusniyarov, Marat M

    2015-10-26

    Spin-crossover metal complexes are highly promising magnetic molecular switches for prospective molecule-based devices. The spin-crossover molecular photoswitches developed so far operate either at very low temperatures or in the liquid phase, which hinders practical applications. Herein, we present a molecular spin-crossover iron(II) complex that can be switched between paramagnetic high-spin and diamagnetic low-spin states with light at room temperature in the solid state. The reversible photoswitching is induced by alternating irradiation with ultraviolet and visible light and proceeds at the molecular level. PMID:26480333

  19. Making classical ground-state spin computing fault-tolerant.

    PubMed

    Crosson, I J; Bacon, D; Brown, K R

    2010-09-01

    We examine a model of classical deterministic computing in which the ground state of the classical system is a spatial history of the computation. This model is relevant to quantum dot cellular automata as well as to recent universal adiabatic quantum computing constructions. In its most primitive form, systems constructed in this model cannot compute in an error-free manner when working at nonzero temperature. However, by exploiting a mapping between the partition function for this model and probabilistic classical circuits we are able to show that it is possible to make this model effectively error-free. We achieve this by using techniques in fault-tolerant classical computing and the result is that the system can compute effectively error-free if the temperature is below a critical temperature. We further link this model to computational complexity and show that a certain problem concerning finite temperature classical spin systems is complete for the complexity class Merlin-Arthur. This provides an interesting connection between the physical behavior of certain many-body spin systems and computational complexity. PMID:21230024

  20. Quantum computation mediated by ancillary qudits and spin coherent states

    NASA Astrophysics Data System (ADS)

    Proctor, Timothy J.; Dooley, Shane; Kendon, Viv

    2015-01-01

    Models of universal quantum computation in which the required interactions between register (computational) qubits are mediated by some ancillary system are highly relevant to experimental realizations of a quantum computer. We introduce such a universal model that employs a d -dimensional ancillary qudit. The ancilla-register interactions take the form of controlled displacements operators, with a displacement operator defined on the periodic and discrete lattice phase space of a qudit. We show that these interactions can implement controlled phase gates on the register by utilizing geometric phases that are created when closed loops are traversed in this phase space. The extra degrees of freedom of the ancilla can be harnessed to reduce the number of operations required for certain gate sequences. In particular, we see that the computational advantages of the quantum bus (qubus) architecture, which employs a field-mode ancilla, are also applicable to this model. We then explore an alternative ancilla-mediated model which employs a spin ensemble as the ancillary system and again the interactions with the register qubits are via controlled displacement operators, with a displacement operator defined on the Bloch sphere phase space of the spin coherent states of the ensemble. We discuss the computational advantages of this model and its relationship with the qubus architecture.

  1. Mesoscopic Superposition States Generated by Synthetic Spin-Orbit Interaction in Fock-State Lattices

    NASA Astrophysics Data System (ADS)

    Wang, Da-Wei; Cai, Han; Liu, Ren-Bao; Scully, Marlan O.

    2016-06-01

    Mesoscopic superposition states of photons can be prepared in three cavities interacting with the same two-level atom. By periodically modulating the three cavity frequencies around the transition frequency of the atom with a 2 π /3 phase difference, the time reversal symmetry is broken and an optical circulator is generated with chiralities depending on the quantum state of the atom. A superposition of the atomic states can guide photons from one cavity to a mesoscopic superposition of the other two cavities. The physics can be understood in a finite spin-orbit-coupled Fock-state lattice where the atom and the cavities carry the spin and the orbit degrees of freedom, respectively. This scheme can be realized in circuit QED architectures and provides a new platform for exploring quantum information and topological physics in novel lattices.

  2. Mesoscopic Superposition States Generated by Synthetic Spin-Orbit Interaction in Fock-State Lattices.

    PubMed

    Wang, Da-Wei; Cai, Han; Liu, Ren-Bao; Scully, Marlan O

    2016-06-01

    Mesoscopic superposition states of photons can be prepared in three cavities interacting with the same two-level atom. By periodically modulating the three cavity frequencies around the transition frequency of the atom with a 2π/3 phase difference, the time reversal symmetry is broken and an optical circulator is generated with chiralities depending on the quantum state of the atom. A superposition of the atomic states can guide photons from one cavity to a mesoscopic superposition of the other two cavities. The physics can be understood in a finite spin-orbit-coupled Fock-state lattice where the atom and the cavities carry the spin and the orbit degrees of freedom, respectively. This scheme can be realized in circuit QED architectures and provides a new platform for exploring quantum information and topological physics in novel lattices. PMID:27314706

  3. Strong Suppression of the Spin Hall Effect in the Spin Glass State

    NASA Astrophysics Data System (ADS)

    Niimi, Y.; Kimata, M.; Omori, Y.; Gu, B.; Ziman, T.; Maekawa, S.; Fert, A.; Otani, Y.

    2015-11-01

    We have measured spin Hall effects in spin glass metals, CuMnBi alloys, with the spin absorption method in the lateral spin valve structure. Far above the spin glass temperature Tg where the magnetic moments of Mn impurities are randomly frozen, the spin Hall angle of a CuMnBi ternary alloy is as large as that of a CuBi binary alloy. Surprisingly, however, it starts to decrease at about 4 Tg and becomes as little as 7 times smaller at 0.5 Tg. A similar tendency was also observed in anomalous Hall effects in the ternary alloys. We propose an explanation in terms of a simple model considering the relative dynamics between the localized moment and the conduction electron spin.

  4. Ground-state energies of the nonlinear sigma model and the Heisenberg spin chains

    NASA Technical Reports Server (NTRS)

    Zhang, Shoucheng; Schulz, H. J.; Ziman, Timothy

    1989-01-01

    A theorem on the O(3) nonlinear sigma model with the topological theta term is proved, which states that the ground-state energy at theta = pi is always higher than the ground-state energy at theta = 0, for the same value of the coupling constant g. Provided that the nonlinear sigma model gives the correct description for the Heisenberg spin chains in the large-s limit, this theorem makes a definite prediction relating the ground-state energies of the half-integer and the integer spin chains. The ground-state energies obtained from the exact Bethe ansatz solution for the spin-1/2 chain and the numerical diagonalization on the spin-1, spin-3/2, and spin-2 chains support this prediction.

  5. Pure and random quantum Ising chain: Shannon and Rényi entropies of the ground state via real space renormalization

    NASA Astrophysics Data System (ADS)

    Monthus, Cécile

    2015-04-01

    The Shannon and the Rényi entropies of the ground state wavefunction in the pure and in the random quantum Ising chain are studied via the self-dual Fernandez-Pacheco real-space renormalization procedure. In particular, we analyze the critical behavior of the leading extensive term at the quantum phase transition : the derivative with respect to the control parameter is found to be logarithmically divergent in the pure case and to display a cusp singularity in the random case. This cusp singularity for the random case is also derived via the Strong Disorder Renormalization approach.

  6. Spin-Wave Diode

    NASA Astrophysics Data System (ADS)

    Lan, Jin; Yu, Weichao; Wu, Ruqian; Xiao, Jiang

    2015-10-01

    A diode, a device allowing unidirectional signal transmission, is a fundamental element of logic structures, and it lies at the heart of modern information systems. The spin wave or magnon, representing a collective quasiparticle excitation of the magnetic order in magnetic materials, is a promising candidate for an information carrier for the next-generation energy-saving technologies. Here, we propose a scalable and reprogrammable pure spin-wave logic hardware architecture using domain walls and surface anisotropy stripes as waveguides on a single magnetic wafer. We demonstrate theoretically the design principle of the simplest logic component, a spin-wave diode, utilizing the chiral bound states in a magnetic domain wall with a Dzyaloshinskii-Moriya interaction, and confirm its performance through micromagnetic simulations. Our findings open a new vista for realizing different types of pure spin-wave logic components and finally achieving an energy-efficient and hardware-reprogrammable spin-wave computer.

  7. Liquid ground state, gap, and excited states of a strongly correlated spin chain.

    PubMed

    Lesanovsky, Igor

    2012-03-01

    We present an exact solution of an experimentally realizable and strongly interacting one-dimensional spin system which is a limiting case of a quantum Ising model with long range interaction in a transverse and longitudinal field. Pronounced quantum fluctuations lead to a strongly correlated liquid ground state. For open boundary conditions the ground state manifold consists of four degenerate sectors whose quantum numbers are determined by the orientation of the edge spins. Explicit expressions for the entanglement properties, the exact excitation gap, as well as the exact wave functions for a couple of excited states are analytically derived and discussed. We outline how this system can be experimentally realized in a lattice gas of Rydberg atoms. PMID:22463419

  8. Spin eigen-states of Dirac equation for quasi-two-dimensional electrons

    SciTech Connect

    Eremko, Alexander; Brizhik, Larissa; Loktev, Vadim

    2015-10-15

    Dirac equation for electrons in a potential created by quantum well is solved and the three sets of the eigen-functions are obtained. In each set the wavefunction is at the same time the eigen-function of one of the three spin operators, which do not commute with each other, but do commute with the Dirac Hamiltonian. This means that the eigen-functions of Dirac equation describe three independent spin eigen-states. The energy spectrum of electrons confined by the rectangular quantum well is calculated for each of these spin states at the values of energies relevant for solid state physics. It is shown that the standard Rashba spin splitting takes place in one of such states only. In another one, 2D electron subbands remain spin degenerate, and for the third one the spin splitting is anisotropic for different directions of 2D wave vector.

  9. Perfect state transfers by selective quantum interferences within complex spin networks

    NASA Astrophysics Data System (ADS)

    Álvarez, Gonzalo A.; Mishkovsky, Mor; Danieli, Ernesto P.; Levstein, Patricia R.; Pastawski, Horacio M.; Frydman, Lucio

    2010-06-01

    We present a method that implements directional, perfect state transfers within a branched spin network by exploiting quantum interferences in the time domain. This method provides a tool for isolating subsystems from a large and complex one. Directionality is achieved by interrupting the spin-spin coupled evolution with periods of free Zeeman evolutions, whose timing is tuned to be commensurate with the relative phases accrued by specific spin pairs. This leads to a resonant transfer between the chosen qubits and to a detuning of all remaining pathways in the network, using only global manipulations. Since the transfer is perfect when the selected pathway is mediated by two or three spins, distant state transfers over complex networks can be achieved by successive recouplings among specific pairs or triads of spins. These effects are illustrated with a quantum simulator involving C13 NMR on leucine’s backbone; a six-spin network.

  10. Bipolar spin blockade and coherent state superpositions in a triple quantum dot.

    PubMed

    Busl, M; Granger, G; Gaudreau, L; Sánchez, R; Kam, A; Pioro-Ladrière, M; Studenikin, S A; Zawadzki, P; Wasilewski, Z R; Sachrajda, A S; Platero, G

    2013-04-01

    Spin qubits based on interacting spins in double quantum dots have been demonstrated successfully. Readout of the qubit state involves a conversion of spin to charge information, which is universally achieved by taking advantage of a spin blockade phenomenon resulting from Pauli's exclusion principle. The archetypal spin blockade transport signature in double quantum dots takes the form of a rectified current. At present, more complex spin qubit circuits including triple quantum dots are being developed. Here we show, both experimentally and theoretically, that in a linear triple quantum dot circuit the spin blockade becomes bipolar with current strongly suppressed in both bias directions and also that a new quantum coherent mechanism becomes relevant. In this mechanism, charge is transferred non-intuitively via coherent states from one end of the linear triple dot circuit to the other, without involving the centre site. Our results have implications for future complex nanospintronic circuits. PMID:23416792

  11. Bipolar spin blockade and coherent state superpositions in a triple quantum dot

    NASA Astrophysics Data System (ADS)

    Busl, M.; Granger, G.; Gaudreau, L.; Sánchez, R.; Kam, A.; Pioro-Ladrière, M.; Studenikin, S. A.; Zawadzki, P.; Wasilewski, Z. R.; Sachrajda, A. S.; Platero, G.

    2013-04-01

    Spin qubits based on interacting spins in double quantum dots have been demonstrated successfully. Readout of the qubit state involves a conversion of spin to charge information, which is universally achieved by taking advantage of a spin blockade phenomenon resulting from Pauli's exclusion principle. The archetypal spin blockade transport signature in double quantum dots takes the form of a rectified current. At present, more complex spin qubit circuits including triple quantum dots are being developed. Here we show, both experimentally and theoretically, that in a linear triple quantum dot circuit the spin blockade becomes bipolar with current strongly suppressed in both bias directions and also that a new quantum coherent mechanism becomes relevant. In this mechanism, charge is transferred non-intuitively via coherent states from one end of the linear triple dot circuit to the other, without involving the centre site. Our results have implications for future complex nanospintronic circuits.

  12. Spin state transition in the active center of the hemoglobin molecule: DFT + DMFT study

    NASA Astrophysics Data System (ADS)

    Novoselov, D.; Korotin, Dm. M.; Anisimov, V. I.

    2016-05-01

    An ab initio study of electronic and spin configurations of the iron ion in the active center of the human hemoglobin molecule is presented. With a combination of the Density Functional Theory (DFT) method and the Dynamical Mean Field Theory (DMFT) approach, the spin state transition description in the iron ion during the oxidation process is significantly improved in comparison with previous attempts. It was found that the origin of the iron ion local moment behavior both for the high-spin and for the low-spin states in the hemoglobin molecule is caused by the presence of a mixture of several atomic states with comparable statistical probability.

  13. Spin polarized bound states in the continuum in open Aharonov-Bohm rings with the Rashba spin-orbit interaction.

    PubMed

    Bulgakov, Evgeny N; Sadreev, Almas F

    2016-07-01

    We consider the trapping of electrons with a definite spin polarization by bound states in the continuum (BSC) in the open Aharonov-Bohm rings in the presence of the Rashba spin-orbit interaction (RSOI). Neglecting the Zeeman term we show the existence of BSCs in the one-dimensional ring when the eigenstates of the closed ring are doubly degenerate. With account of the Zeeman term BSCs occur only at the points of threefold degeneracy. The BSCs are found in the parametric space of flux and RSOI strength in close pairs with opposite spin polarization. Thereby the spin polarization of electrons transmitted through the ring can be altered by minor variation of magnetic or electric field at the vicinity of these pairs. Numerical simulations of the two-dimensional open ring show similar results for the BSCs. Encircling the BSC points in the parametric space of the flux and the RSOI constant gives rise to a geometric phase. PMID:27165662

  14. High-sensitivity single NV magnetometry by spin-to-charge state mapping

    NASA Astrophysics Data System (ADS)

    Jaskula, Jean-Christophe; Shields, Brendan; Bauch, Erik; Lukin, Mikhail; Walsworth, Ronald; Trifonov, Alexei

    2015-05-01

    Nitrogen-Vacancy (NV) centers in diamond are atom-like quantum system in a solid state matrix whom its structure allows optical readout of the electronic spin. However, the optimal duration of optical readout is limited by a singlet state lifetime making single shot spin readout out of reach. On the other side, the NV center charge state readout can be extremely efficient (up to 99% fidelity) by using excitation at 594 nm. We will present a new method of spin readout utilizing a spin-depending photoionization process to map the electronic spin state of the NV onto the its charge state. Moreover, pre-selection on the charged state allows to minimize data acquisition time. This scheme improves single NV AC magnetometry by a factor of 5 and will benefit other single NV center experiments as well.

  15. Orbital-symmetry-selective spin characterization of Dirac-cone-like state on W(110)

    NASA Astrophysics Data System (ADS)

    Miyamoto, K.; Wortelen, H.; Mirhosseini, H.; Okuda, T.; Kimura, A.; Iwasawa, H.; Shimada, K.; Henk, J.; Donath, M.

    2016-04-01

    The surface of W(110) exhibits a spin-orbit-induced Dirac-cone-like surface state, which is of mainly dz2 orbital character near Γ ¯, although it is strongly influenced by the twofold C2 v surface symmetry. Its distinctive k-dependent spin polarization along Γ ¯H ¯ is revealed by spin- and angle-resolved photoemission excited with p - and s -polarized light. The spin texture of the surface state is found to change sign upon switching from p - to s -polarized light. Based on electronic-structure calculations, this behavior is explained by the orbital composition of the Dirac-cone-like state. The dominant part of the state has even mirror symmetry and is excited by p -polarized light. A minor part with odd symmetry is excited by s -polarized light and exhibits a reversed spin polarization. Our study demonstrates in which way spin-orbit interaction combines the spin degree of freedom with the orbital degree of freedom and opens a way to manipulate the spin information gathered from the Dirac-cone-like surface state by light. Our results prove that "spin control" is not restricted to topological surface states with p -type orbital symmetry in topological insulators.

  16. Magnetic-field-induced density of states in Mg B2 : Spin susceptibility measured by conduction-electron spin resonance

    NASA Astrophysics Data System (ADS)

    Simon, F.; Jánossy, A.; Fehér, T.; Murányi, F.; Garaj, S.; Forró, L.; Petrovic, C.; Bud'Ko, S.; Ribeiro, R. A.; Canfield, P. C.

    2005-07-01

    The magnetic-field dependence of the electron spin susceptibility χs was measured in the superconducting state of high-purity MgB2 fine powders from the intensity of the conduction-electron spin resonance at 3.8, 9.4, and 35GHz . The measurements confirm that a large part of the density of states is restored at low temperatures at fields below 1T in qualitative agreement with the closing of the π band gaps in the two-band model. However, the increase of χs with field and temperature is larger than expected from current superconductor models of MgB2 .

  17. A quantum phase switch between a single solid-state spin and a photon

    NASA Astrophysics Data System (ADS)

    Sun, Shuo; Kim, Hyochul; Solomon, Glenn S.; Waks, Edo

    2016-06-01

    Interactions between single spins and photons are essential for quantum networks and distributed quantum computation. Achieving spin–photon interactions in a solid-state device could enable compact chip-integrated quantum circuits operating at gigahertz bandwidths. Many theoretical works have suggested using spins embedded in nanophotonic structures to attain this high-speed interface. These proposals implement a quantum switch where the spin flips the state of the photon and a photon flips the spin state. However, such a switch has not yet been realized using a solid-state spin system. Here, we report an experimental realization of a spin–photon quantum switch using a single solid-state spin embedded in a nanophotonic cavity. We show that the spin state strongly modulates the polarization of a reflected photon, and a single reflected photon coherently rotates the spin state. These strong spin–photon interactions open up a promising direction for solid-state implementations of high-speed quantum networks and on-chip quantum information processors using nanophotonic devices.

  18. Observations of high spin states in {sup 179}Au

    SciTech Connect

    Carpenter, M.P.; Ahmad, I.; Blumenthal, D.J.

    1995-08-01

    As part of a current study on the properties of the {pi} i{sub 13/2} intruder state in the A = 175-190 region, we conducted an experiment at ATLAS to observe high spin states in {sup 179}Au utilizing the reaction {sup 144}Sm({sup 40}Ar,p4n) at beam energies of 207 MeV and 215 MeV. To aid in the identification of {sup 179}Au, and to filter out the large amount of events from fission by-products, the Fragment Mass Analyzer was utilized in conjunction with ten Compton-suppression germanium detectors. In total, 11 x 10{sup 6} {gamma}-{gamma} and 4 x 10{sup 5} {gamma}-recoil events were collected. By comparing {gamma}-rays in coincidence with an A = 179 recoil mass gate and {gamma}-rays in coincidence with Au K{alpha} and K{beta} X-rays, ten {gamma}-rays were identified as belonging to {sup 179}Au. Based on {gamma}-ray coincidence relationships and on comparisons with neighboring odd-A Au nuclei, we constructed a tentative level scheme and assigned a rotational-like sequence to the {pi} i{sub 13/2} proton configuration.

  19. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet.

    PubMed

    Fu, Mingxuan; Imai, Takashi; Han, Tian-Heng; Lee, Young S

    2015-11-01

    The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χ(kagome), deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of χ(kagome) that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap. PMID:26542565

  20. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet

    DOE PAGESBeta

    Fu, Mingxuan; Imai, Takahashi; Han, Tian -Heng; Lee, Young S.

    2015-11-06

    Here, the kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χkagome, deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with themore » magnetic field dependence of χkagome that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.« less

  1. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet

    NASA Astrophysics Data System (ADS)

    Fu, Mingxuan; Imai, Takashi; Han, Tian-Heng; Lee, Young S.

    2015-11-01

    The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χkagome, deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of χkagome that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.

  2. Aging and memory effects in the spin jam states of densely populated frustrated magnets

    NASA Astrophysics Data System (ADS)

    Samarakoon, Anjana; Lee, Seung-Hun; Sato, Taku; Zhou, Haidong; Sinclair, Ryan; Yang, Junjie; Chen, Tianran; Chern, Gia-Wei; Klich, Israel

    Defects and randomness has been largely studied as the key mechanism of glassiness find in a dilute magnetic system. Even though the same argument has also been made to explain the spin glass like properties in dense frustrated magnets, the existence of a glassy state arise intrinsically from a defect free spin system, far from the conventional dilute limit with different mechanisms such as quantum fluctuations and topological features, has been theoretically proposed recently. We have studied field effects on zero-field cooled and field cooled susceptibility bifurcation and memory effects below freezing transition, of three different densely populated frustrated magnets which glassy states we call spin jam, and a conventional dilute spin glass. Our data show common behaviors among the spin jam states, which is distinct from that of the conventional spin glass. We have also performed Monte Carlo simulations to understand the nature of their energy landscapes.

  3. Spin polarized electronic states and spin textures at the surface of oxygen-deficient SrTiO3

    NASA Astrophysics Data System (ADS)

    Jeschke, Harald O.; Altmeyer, Michaela; Rozenberg, Marcelo; Gabay, Marc; Valenti, Roser

    We investigate the electronic structure and spin texture at the (001) surface of SrTiO3 in the presence of oxygen vacancies by means of ab initio density functional theory (DFT) calculations of slabs. Relativistic non-magnetic DFT calculations exhibit Rashba-like spin winding with a characteristic energy scale ~ 10 meV. However, when surface magnetism on the Ti ions is included, bands become spin-split with an energy difference ~ 100 meV at the Γ point. This energy scale is comparable to the observations in SARPES experiments performed on the two-dimensional electronic states confined near the (001) surface of SrTiO3. We find the spin polarized state to be the ground state of the system, and while magnetism tends to suppress the effects of the relativistic Rashba interaction, signatures of it are still clearly visible in terms of complex spin textures. We gratefully acknowledge financial support from the Deutsche Forschungsgemeinschaft through grants SFB/TR 49 and FOR 1346.

  4. Memory-built-in quantum cloning in a hybrid solid-state spin register

    PubMed Central

    Wang, W.-B.; Zu, C.; He, L.; Zhang, W.-G.; Duan, L.-M.

    2015-01-01

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude. The realization of a cloning machine with built-in quantum memory provides a key step for application of quantum cloning in quantum information science. PMID:26178617

  5. Memory-built-in quantum cloning in a hybrid solid-state spin register

    NASA Astrophysics Data System (ADS)

    Wang, Weibin; Zu, Chong; He, Li; Zhang, Wengang; Duan, Luming

    2015-05-01

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude, and making it an ideal memory qubit. Our experiment is based on control of an individual nitrogen vacancy (NV) center in the diamond, which is a diamond defect that attracts strong interest in recent years with great potential for implementation of quantum information protocols.

  6. Memory-built-in quantum cloning in a hybrid solid-state spin register

    NASA Astrophysics Data System (ADS)

    Wang, W.-B.; Zu, C.; He, L.; Zhang, W.-G.; Duan, L.-M.

    2015-07-01

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude. The realization of a cloning machine with built-in quantum memory provides a key step for application of quantum cloning in quantum information science.

  7. Memory-built-in quantum cloning in a hybrid solid-state spin register.

    PubMed

    Wang, W-B; Zu, C; He, L; Zhang, W-G; Duan, L-M

    2015-01-01

    As a way to circumvent the quantum no-cloning theorem, approximate quantum cloning protocols have received wide attention with remarkable applications. Copying of quantum states to memory qubits provides an important strategy for eavesdropping in quantum cryptography. We report an experiment that realizes cloning of quantum states from an electron spin to a nuclear spin in a hybrid solid-state spin register with near-optimal fidelity. The nuclear spin provides an ideal memory qubit at room temperature, which stores the cloned quantum states for a millisecond under ambient conditions, exceeding the lifetime of the original quantum state carried by the electron spin by orders of magnitude. The realization of a cloning machine with built-in quantum memory provides a key step for application of quantum cloning in quantum information science. PMID:26178617

  8. Pi topology and spin alignment in unique photoexcited triplet and quintet states arising from four unpaired electrons of an organic spin system.

    PubMed

    Teki, Yoshio; Toichi, Tetuya; Nakajima, Satoru

    2006-03-01

    Syntheses, electronic structures in the ground state, unique photoexcited states, and spin alignment are reported for novel biradical 1, which was designed as an ideal model compound to investigate photoinduced spin alignment in the excited state. Electron spin resonance (ESR), time-resolved ESR (TRESR), and laser-excitation pulsed ESR experiments were carried out. The magnetic properties were examined with a SQUID magnetometer. In the electronic ground state, two radical moieties interact very weakly (almost no interaction) with each other through the closed-shell diphenylanthracene spin coupler. On photoirradiation, a novel lowest photoexcited state with the intermediate spin (S = 1) arising from four unpaired electrons with low-lying quintet (S = 2) photoexcited state was detected. The unique triplet state has an interesting electronic structure, the D value of which is reduced by antiferromagnetic spin alignment between two radical spins through the excited triplet spin coupler. The general theoretical predictions of the spin alignment and the reduction of the fine-structure splitting of the triplet bis(radical) systems are presented. The fine-structure splitting of the unique photoexcited triplet state of 1, as well as the existence of the low-lying quintet state, is interpreted well on the basis of theoretical predictions. Details of the spin alignment in the photoexcited states are discussed. PMID:16372362

  9. Solid-state characterization of optically pure (+)Dihydromyricetin extracted from Ampelopsis grossedentata leaves.

    PubMed

    Wang, Chenguang; Xiong, Wei; Reddy Perumalla, Sathyanarayana; Fang, Jianguo; Calvin Sun, Changquan

    2016-09-10

    Dihydromyricetin (DMY) is a natural flavanol compound isolated from a traditional Chinese medicine, Ampelopsis grossedentata. Despite that optically pure (+)DMY is desired for treating chronic pharyngitis and alcohol use disorders, only DMY racemate is commercially available due to prolonged exposure time to high temperature and the presence of metal ions during industrial extraction, which cause racemization of the homochiral (+)DMY. We have developed an extraction method for successfully obtain optically pure (+)DMY. We have further assessed the physicochemical properties of the two phases using PXRD, DSC, TGA, FTIR, and moisture sorption. Among them, PXRD and FT-IR are suitable for quickly distinguishing homochiral (+)DMY from racemic (±)DMY. Lastly, with the aid of cocrystallization with theophylline, the absolute configuration of homochiral (+)DMY was identified to be (2R, 3R). PMID:27418561

  10. Charge, spin, and lattice effects in the spin-Peierls ground state of MEM(TCNQ)2

    NASA Astrophysics Data System (ADS)

    Poirier, Mario; de Lafontaine, Mathieu; Bourbonnais, Claude; Pouget, Jean-Paul

    2013-12-01

    We report an investigation of charge, spin, and lattice effects in the spin-Peierls state of the organic compound MEM(TCNQ)2. The 16.5-GHz dielectric function along the chain axis shows an enhancement below the spin-Peierls transition temperature near 18 K consistent with the charge coupling to the elastic strain involved in the transition. The velocity of two elastic modes perpendicular to the chain axis presents anomalies at the transition, which can be explained with a Landau free-energy model including a linear-quadratic coupling energy term between the appropriate elastic strain e and the spin-Peierls magnetic gap Δq. The analysis of the dielectric and elastic features aims toward an order parameter with an associated critical exponent β ˜ 0.36, which is similar to the three-dimensional behavior seen in other spin-Peierls materials. All these effects studied in a magnetic field up to 18 Teslas appear also compatible with a mean-field model of a quasi-one-dimensional spin-Peierls system.

  11. On the accuracy of the state space restriction approximation for spin dynamics simulations

    NASA Astrophysics Data System (ADS)

    Karabanov, Alexander; Kuprov, Ilya; Charnock, G. T. P.; van der Drift, Anniek; Edwards, Luke J.; Köckenberger, Walter

    2011-08-01

    We present an algebraic foundation for the state space restriction approximation in spin dynamics simulations and derive applicability criteria as well as minimal basis set requirements for practically encountered simulation tasks. The results are illustrated with nuclear magnetic resonance (NMR), electron spin resonance (ESR), dynamic nuclear polarization (DNP), and spin chemistry simulations. It is demonstrated that state space restriction yields accurate results in systems where the time scale of spin relaxation processes approximately matches the time scale of the experiment. Rigorous error bounds and basis set requirements are derived.

  12. Zero-Magnetic-Field Spin Splitting of Polaron's Ground State Energy Induced by Rashba Spin-Orbit Interaction

    NASA Astrophysics Data System (ADS)

    Liu, Jia; Xiao, Jing-Ling

    2006-10-01

    We study theoretically the ground state energy of a polaron near the interface of a polar-polar semiconductor by considering the Rashba spin-orbit (SO) coupling with the Lee-Low-Pines intermediate coupling method. Our numerical results show that the Rashba SO interaction originating from the inversion asymmetry in the heterostructure splits the ground state energy of the polaron. The electron areal density and vector dependence of the ratio of the SO interaction to the total ground state energy or other energy composition are obvious. One can see that even without any external magnetic field, the ground state energy can be split by the Rashba SO interaction, and this split is not a single but a complex one. Since the presents of the phonons, whose energy gives negative contribution to the polaron's, the spin-splitting states of the polaron are more stable than electron's.

  13. Are Very Small Emission Quantum Yields Characteristic of Pure Metal-to-Ligand Charge-Transfer Excited States of Ruthenium(II)-(Acceptor Ligand) Chromophores?

    PubMed

    Tsai, Chia Nung; Mazumder, Shivnath; Zhang, Xiu Zhu; Schlegel, H Bernhard; Chen, Yuan Jang; Endicott, John F

    2016-08-01

    Metal to ligand charge-transfer (MLCT) excited state emission quantum yields, ϕem, are reported in 77 K glasses for a series of pentaammine and tetraammine ruthenium(II) complexes with monodentate aromatic acceptor ligands (Ru-MDA) such as pyridine and pyrazine. These quantum yields are only about 0.2-1% of those found for their Ru-bpy (bpy = 2,2'-bipyridine) analogs in similar excited state energy ranges (hνem). The excited state energy dependencies of the emission intensity are characterized by mean radiative decay rate constants, kRAD, resolved from ϕem/τobs = kRAD (τobs = the observed emission decay lifetime; τobs(-1) = kRAD + kNRD; kNRD = nonradiative decay rate constant). Except for the Ru-pz chromophores in alcohol glasses, the values of kNRD for the Ru-MDA chromophores are slightly smaller, and their dependences on excited state energies are very similar to those of related Ru-bpy chromophores. In principle, one expects kRAD to be proportional to the product of (hνem)(3) and the square of the transition dipole moment (Me,g).(2) However, from experimental studies of Ru-bpy chromophores, an additional hνem dependence has been found that originates in an intensity stealing from a higher energy excited state with a much larger value of Me,g. This additional hνem dependence is not present in the kRAD energy dependence for Ru-MDA chromophores in the same energy regime. Intensity stealing in the phosphorescence of these complexes is necessary since the triplet-to-singlet transition is only allowed through spin-orbit coupling and since the density functional theory modeling implicates configurational mixing between states in the triplet spin manifold; this is treated by setting Me,g equal to the product of a mixing coefficient and the difference between the molecular dipole moments of the states involved, which implicates an experimental first order dependence of kRAD on hνem. The failure to observe intensity stealing for the Ru-MDA complexes suggests

  14. All-optical formation of coherent dark states of silicon-vacancy spins in diamond.

    PubMed

    Pingault, Benjamin; Becker, Jonas N; Schulte, Carsten H H; Arend, Carsten; Hepp, Christian; Godde, Tillmann; Tartakovskii, Alexander I; Markham, Matthew; Becher, Christoph; Atatüre, Mete

    2014-12-31

    Spin impurities in diamond can be versatile tools for a wide range of solid-state-based quantum technologies, but finding spin impurities that offer sufficient quality in both photonic and spin properties remains a challenge for this pursuit. The silicon-vacancy center has recently attracted much interest because of its spin-accessible optical transitions and the quality of its optical spectrum. Complementing these properties, spin coherence is essential for the suitability of this center as a spin-photon quantum interface. Here, we report all-optical generation of coherent superpositions of spin states in the ground state of a negatively charged silicon-vacancy center using coherent population trapping. Our measurements reveal a characteristic spin coherence time, T2*, exceeding 45 nanoseconds at 4 K. We further investigate the role of phonon-mediated coupling between orbital states as a source of irreversible decoherence. Our results indicate the feasibility of all-optical coherent control of silicon-vacancy spins using ultrafast laser pulses. PMID:25615329

  15. Generic helical edge states due to Rashba spin-orbit coupling in a topological insulator

    NASA Astrophysics Data System (ADS)

    Ortiz, Laura; Molina, Rafael A.; Platero, Gloria; Lunde, Anders Mathias

    2016-05-01

    We study the helical edge states of a two-dimensional topological insulator without axial spin symmetry due to the Rashba spin-orbit interaction. Lack of axial spin symmetry can lead to so-called generic helical edge states, which have energy-dependent spin orientation. This opens the possibility of inelastic backscattering and thereby nonquantized transport. Here we find analytically the new dispersion relations and the energy dependent spin orientation of the generic helical edge states in the presence of Rashba spin-orbit coupling within the Bernevig-Hughes-Zhang model, for both a single isolated edge and for a finite width ribbon. In the single-edge case, we analytically quantify the energy dependence of the spin orientation, which turns out to be weak for a realistic HgTe quantum well. Nevertheless, finite size effects combined with Rashba spin-orbit coupling result in two avoided crossings in the energy dispersions, where the spin orientation variation of the edge states is very significantly increased for realistic parameters. Finally, our analytical results are found to compare well to a numerical tight-binding regularization of the model.

  16. Spin Polarization of the ν=1 Quantum Hall State Via Optical Spectroscopy

    NASA Astrophysics Data System (ADS)

    Goldberg, B. B.

    1996-03-01

    Recent theoretical work has shown that the response of a 2DES with small g-factor in the spin-polarized state (ν=1) to a change of one quantum of magnetic flux is not a single-particle spin-flip excitation, but rather a macroscopic spin object called a Skyrmion or charged spin-texture excitation (CSTE).(S. L. Sondhi, A. Karlhede, S. A. Kivelson, and E. H. Rezayi, Phys. Rev. B 47), 16419 (1993); H. A. Fertig, L. Brey, R. Cote, and A. H. MacDonald, Phys. Rev. B 50, 11018 (1994) Evidence of these excitations have been recently observed in NMR and in tilted-field transport measurements.(S. E. Barrett, G. Dabbagh, L. N. Pfeiffer, K. W. West, and Z. Tycko, Phys. Rev. Lett. 74), 5112 (1995); A. Schmeller, J. P. Eisenstein, L. N. Pfeiffer, K. W. West, LANL Cond-mat preprint 9506133. They consist of a radial spin density distribution that is reversed at the center but gradually heals to the spin background over a distance of many magnetic lengths. With each particle in a nearly spin-aligned neighborhood, the exchange contribution lowers the energy of the CSTE relative to a single flipped spin. We present an experimental observation of Skyrmions in GaAs through the dramatic reduction in the degree of spin-polarization when the Fermi energy moves off the mid-point of the spin-gap of the lowest Landau level, ν=1. The degree of electron spin polarization as a function of ν is measured through interband magneto-absorption spectroscopy which distinguish the occupancy of the two electron spin-states. The spectra show quenching of absorption to the lower energy, spin-up electron band directly correlated to an increase in the higher energy, spin-down absorption at ν=1. This indicates the spin-up state fills with electrons while the spin-down state empties, providing a large spin-polarization Sz which exhibits a pronounced, symmetric decay when ν deviates from 1. The data provide a measurement of the absolute electron spin and are evidence for the presence of Skyrmion

  17. Quantum Spin Hall States in Stanene/Ge(111)

    PubMed Central

    Fang, Yimei; Huang, Zhi-Quan; Hsu, Chia-Hsiu; Li, Xiaodan; Xu, Yixu; Zhou, Yinghui; Wu, Shunqing; Chuang, Feng-Chuan; Zhu, Zi-Zhong

    2015-01-01

    For topological insulators to be implemented in practical applications, it is a prerequisite to select suitable substrates that are required to leave insulators’ nontrivial properties and sizable opened band gaps (due to spin-orbital couplings) unaltered. Using ab initio calculations, we predict that Ge(111) surface qualified as a candidate to support stanene sheets, because the band structure of √3 × √3 stanene/Ge(111) (2 × 2) surface displays a typical Dirac cone at Γ point in the vicinity of the Fermi level. Aided with the result of Z2 invariant calculations, a √3 × √3 stanene/Ge(111) (2 × 2) system has been proved to sustain the nontrivial topological phase, with the prove being confirmed by the edge state calculations of stanene ribbons. This finding can serve as guidance for epitaxial growth of stanene on substrate and render stanene feasible for practical use as a topological insulator. PMID:26374077

  18. Surface-induced spin state locking of the [Fe(H2B(pz)2)2(bipy)] spin crossover complex

    NASA Astrophysics Data System (ADS)

    Beniwal, S.; Zhang, X.; Mu, S.; Naim, A.; Rosa, P.; Chastanet, G.; Létard, J.-F.; Liu, J.; Sterbinsky, G. E.; Arena, D. A.; Dowben, P. A.; Enders, A.

    2016-05-01

    Temperature- and coverage-dependent studies of the Au(1 1 1)-supported spin crossover Fe(II) complex (SCO) of the type [Fe(H2B(pz)2)2(bipy)] with a suite of surface-sensitive spectroscopy and microscopy tools show that the substrate inhibits thermally induced transitions of the molecular spin state, so that both high-spin and low-spin states are preserved far beyond the spin transition temperature of free molecules. Scanning tunneling microscopy confirms that [Fe(H2B(pz)2)2(bipy)] grows as ordered, molecular bilayer islands at sub-monolayer coverage and as disordered film at higher coverage. The temperature dependence of the electronic structure suggest that the SCO films exhibit a mixture of spin states at room temperature, but upon cooling below the spin crossover transition the film spin state is best described as a mix of high-spin and low-spin state molecules of a ratio that is constant. This locking of the spin state is most likely the result of a substrate-induced conformational change of the interfacial molecules, but it is estimated that also the intra-atomic electron–electron Coulomb correlation energy, or Hubbard correlation energy U, could be an additional contributing factor.

  19. Surface-induced spin state locking of the [Fe(H2B(pz)2)2(bipy)] spin crossover complex.

    PubMed

    Beniwal, S; Zhang, X; Mu, S; Naim, A; Rosa, P; Chastanet, G; Létard, J-F; Liu, J; Sterbinsky, G E; Arena, D A; Dowben, P A; Enders, A

    2016-05-25

    Temperature- and coverage-dependent studies of the Au(1 1 1)-supported spin crossover Fe(II) complex (SCO) of the type [Fe(H2B(pz)2)2(bipy)] with a suite of surface-sensitive spectroscopy and microscopy tools show that the substrate inhibits thermally induced transitions of the molecular spin state, so that both high-spin and low-spin states are preserved far beyond the spin transition temperature of free molecules. Scanning tunneling microscopy confirms that [Fe(H2B(pz)2)2(bipy)] grows as ordered, molecular bilayer islands at sub-monolayer coverage and as disordered film at higher coverage. The temperature dependence of the electronic structure suggest that the SCO films exhibit a mixture of spin states at room temperature, but upon cooling below the spin crossover transition the film spin state is best described as a mix of high-spin and low-spin state molecules of a ratio that is constant. This locking of the spin state is most likely the result of a substrate-induced conformational change of the interfacial molecules, but it is estimated that also the intra-atomic electron-electron Coulomb correlation energy, or Hubbard correlation energy U, could be an additional contributing factor. PMID:27121917

  20. Low-temperature Spin-Ice State of Quantum Heisenberg Magnets on Pyrochlore Lattice

    NASA Astrophysics Data System (ADS)

    Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris

    We establish that the isotropic spin-1/2 Heisenberg antiferromagnet on pyrochlore lattice enters a spin-ice state at low, but finite, temperature. Our conclusions are based on results of the bold diagrammatic Monte Carlo simulations that demonstrate good convergence of the skeleton series down to temperature T = J/6. The ``smoking gun'' identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for static spin-spin correlation function between the quantum Heisenberg and classical Heisenberg/Ising models at all accessible temperatures. In particular, at T/J = 1/6, the momentum dependence shows a characteristic bow-tie pattern with pinch points. By numerical analytical continuation method, we also obtain the dynamic structure factor at real frequencies, showing a diffusive spinon dynamics at pinch points and spin wave continuum along the nodal lines.?

  1. Coherent states and nonlinear dynamics of the three state quasi-spin model with soliton solutions

    NASA Astrophysics Data System (ADS)

    Agüero, M.; Alvarado, R.; Frias, M.

    1998-11-01

    In this paper the generalized coherent states defined as points of the coset space {SU(2)}/{U(1)} are used as trial wave functions in order to study the quasi-spin model of the nonlinear ϕ6-theory. In the simple version of the quasi-classical theory deduced from this method a complete integrable system is obtained. In a general context, the ground state and linear spectrum of the nonlinear lattice equation were evaluated. Finally, by analyzing the effective potential, the first and second order phase transitions are shown to exist.

  2. Electrical spin injection and detection in Fe/MgO/Si: influence of interface states

    NASA Astrophysics Data System (ADS)

    Pu, Yong; Beardsley, Jonas; Swartz, Adrain; Odenthal, Patrick; Berger, Andrew; Ko, Dongkyun; Bhallamudi, Vydia; Hammel, Chris; Kawakami, Roland; Johnston-Halperin, Ezekiel; Pelz, Jon

    2012-02-01

    We report electrical spin injection and detection in Fe/MgO/Si tunnel diodes using a 3-terminal (3T) geometry. Analysis of our Hanle curves yields an effective spin life-time of ˜0.1 ns and a spin-RA product ˜1 Mφ*μm^2, both of which are in rough agreement with previous 3T studies. However, according to our analysis the spin-RA is ˜ 6 orders of magnitude larger than expectations for bulk Si, and the 0.1 ns effective spin life-time is much smaller than reported value in Si by ESR or non-local methods. Here we provide a detailed analysis of electrical injection and detection in the 3T geometry. We present an alternative expression for the 3T spin signal than is usually used, and we propose that spin is accumulating in localized states (LS) at the MgO/Si interface rather than just in bulk Si. Incorporating a theory of spin accumulation in LS developed by M. Tran et al (PRL 102, 036601), we propose an energy distribution for the density of localized states, and introduce a model that agrees well with our anomalously large spin-RA and can explain the strong bias dependence of both spin and charge transport.

  3. Feasible Perturbations of Control Systems with Pure State Constraints and Applications to Second-Order Optimality Conditions

    SciTech Connect

    Hoehener, Daniel

    2013-10-15

    We propose second-order necessary optimality conditions for optimal control problems with very general state and control constraints which hold true under weak regularity assumptions on the data. In particular the pure state constraints are general closed sets, the optimal control is supposed to be merely measurable and the dynamics may be discontinuous in the time variable as well. These results are obtained by an approach based on local perturbations of the reference process by second-order tangent directions. This method allows direct and quite simple proofs.

  4. A quantum phase switch between a solid state spin and a photon

    NASA Astrophysics Data System (ADS)

    Sun, Shuo; Kim, Hyochul; Solomon, Glenn; Waks, Edo

    The implementation of quantum network and distributive quantum computation replies on strong interactions between stationary matter qubits and flying photons. The spin of a single electron confined in a quantum dot is considered as a promising matter qubit as it possesses microsecond coherence time and allows picosecond timescale control using optical pulses. The quantum dot spin can also interact with a photon by controlling the optical response of a strongly coupled cavity. In this talk I will discuss our recent work on an experimental realization of a spin-photon quantum phase switch using a single spin in a quantum dot strongly coupled to a photonic crystal cavity. We show large modulation of the cavity reflection spectrum by manipulating the spin states of the quantum dot, which enables us to control the quantum state of a reflected photon. We also show the complementary effect where the presence of a single photon switches the quantum state of the spin. The reported spin-photon quantum phase operation can switch spin or photon states in picoseconds timescale, representing an important step towards GHz semiconductor based quantum logic devices on-a-chip and solid-state implementations of quantum networks.

  5. High spin polarization and the origin of unique ferromagnetic ground state in CuFeSb

    NASA Astrophysics Data System (ADS)

    Sirohi, Anshu; Singh, Chandan K.; Thakur, Gohil S.; Saha, Preetha; Gayen, Sirshendu; Gaurav, Abhishek; Jyotsna, Shubhra; Haque, Zeba; Gupta, L. C.; Kabir, Mukul; Ganguli, Ashok K.; Sheet, Goutam

    2016-06-01

    CuFeSb is isostructural to the ferro-pnictide and chalcogenide superconductors and it is one of the few materials in the family that are known to stabilize in a ferromagnetic ground state. Majority of the members of this family are either superconductors or antiferromagnets. Therefore, CuFeSb may be used as an ideal source of spin polarized current in spin-transport devices involving pnictide and the chalcogenide superconductors. However, for that the Fermi surface of CuFeSb needs to be sufficiently spin polarized. In this paper we report direct measurement of transport spin polarization in CuFeSb by spin-resolved Andreev reflection spectroscopy. From a number of measurements using multiple superconducting tips we found that the intrinsic transport spin polarization in CuFeSb is high (˜47%). In order to understand the unique ground state of CuFeSb and the origin of large spin polarization at the Fermi level, we have evaluated the spin-polarized band structure of CuFeSb through first principles calculations. Apart from supporting the observed 47% transport spin polarization, such calculations also indicate that the Sb-Fe-Sb angles and the height of Sb from the Fe plane are strikingly different for CuFeSb than the equivalent parameters in other members of the same family thereby explaining the origin of the unique ground state of CuFeSb.

  6. Simultaneous generation of two spin-wave-photon entangled states in an atomic ensemble

    NASA Astrophysics Data System (ADS)

    Wu, Yuelong; Tian, Long; Xu, Zhongxiao; Ge, Wei; Chen, Lirong; Li, Shujing; Yuan, Haoxiang; Wen, Yafei; Wang, Hai; Xie, Changde; Peng, Kunchi

    2016-05-01

    Spontaneous Raman scattering (SRS) in atomic ensembles provides a promising method to generate spin-wave-photon entangled states. In the past experiments, a spin-wave-photon entangled state was produced via SRS from an atomic ensemble. Here, we report a scheme of simultaneously generating two spin-wave-photon (atom-photon) entangled states in a cold Rb ensemble via SRS. Based on joint Bell-state measurements on the two photons coming from the two atom-photon entangled sources, respectively, we projected the two stored spin waves into a Bell state and then mapped the quantum memory into a polarization-entangled photon pair. Such a polarization-entangled photon pair can be released on demand and thus the presented scheme has potential application in the preparation of large-size photonic entangled states.

  7. Revisiting spin-lattice relaxation time measurements for dilute spins in high-resolution solid-state NMR spectroscopy

    NASA Astrophysics Data System (ADS)

    Fu, Riqiang; Li, Jun; Cui, Jingyu; Peng, Xinhua

    2016-07-01

    Numerous nuclear magnetic resonance (NMR) measurements of spin-lattice relaxation times (T1S) for dilute spins such as 13C have led to investigations of the motional dynamics of individual functional groups in solid materials. In this work, we revisit the Solomon equations and analyze how the heteronuclear cross relaxation between the dilute S (e.g. 13C) and abundant I (e.g. 1H) spins affects the measured T1S values in solid-state NMR in the absence of 1H saturation during the recovery time. It is found theoretically that at the beginning of the S spin magnetization recovery, the existence of non-equilibrium I magnetization introduces the heteronuclear cross relaxation effect onto the recovery of the S spin magnetization and confirmed experimentally that such a heteronuclear cross relaxation effect results in the recovery overshoot phenomena for the dilute spins when T1S is on the same order of T1H, leading to inaccurate measurements of the T1S values. Even when T1S is ten times larger than T1H, the heteronuclear cross relaxation effect on the measured T1S values is still noticeable. Furthermore, this cross relaxation effect on recovery trajectory of the S spins can be manipulated and even suppressed by preparing the initial I and S magnetization, so as to obtain the accurate T1S values. A sample of natural abundance L-isoleucine powder has been used to demonstrate the T1S measurements and their corresponding measured T1C values under various experimental conditions.

  8. Revisiting spin-lattice relaxation time measurements for dilute spins in high-resolution solid-state NMR spectroscopy.

    PubMed

    Fu, Riqiang; Li, Jun; Cui, Jingyu; Peng, Xinhua

    2016-07-01

    Numerous nuclear magnetic resonance (NMR) measurements of spin-lattice relaxation times (T1S) for dilute spins such as (13)C have led to investigations of the motional dynamics of individual functional groups in solid materials. In this work, we revisit the Solomon equations and analyze how the heteronuclear cross relaxation between the dilute S (e.g. (13)C) and abundant I (e.g. (1)H) spins affects the measured T1S values in solid-state NMR in the absence of (1)H saturation during the recovery time. It is found theoretically that at the beginning of the S spin magnetization recovery, the existence of non-equilibrium I magnetization introduces the heteronuclear cross relaxation effect onto the recovery of the S spin magnetization and confirmed experimentally that such a heteronuclear cross relaxation effect results in the recovery overshoot phenomena for the dilute spins when T1S is on the same order of T1H, leading to inaccurate measurements of the T1S values. Even when T1S is ten times larger than T1H, the heteronuclear cross relaxation effect on the measured T1S values is still noticeable. Furthermore, this cross relaxation effect on recovery trajectory of the S spins can be manipulated and even suppressed by preparing the initial I and S magnetization, so as to obtain the accurate T1S values. A sample of natural abundance l-isoleucine powder has been used to demonstrate the T1S measurements and their corresponding measured T1C values under various experimental conditions. PMID:27187211

  9. Robustness of spin-coupling distributions for perfect quantum state transfer

    SciTech Connect

    Zwick, Analia; Alvarez, Gonzalo A.; Stolze, Joachim; Osenda, Omar

    2011-08-15

    The transmission of quantum information between different parts of a quantum computer is of fundamental importance. Spin chains have been proposed as quantum channels for transferring information. Different configurations for the spin couplings were proposed in order to optimize the transfer. As imperfections in the creation of these specific spin-coupling distributions can never be completely avoided, it is important to find out which systems are optimally suited for information transfer by assessing their robustness against imperfections or disturbances. We analyze different spin coupling distributions of spin chain channels designed for perfect quantum state transfer. In particular, we study the transfer of an initial state from one end of the chain to the other end. We quantify the robustness of different coupling distributions against perturbations and we relate it to the properties of the energy eigenstates and eigenvalues. We find that the localization properties of the systems play an important role for robust quantum state transfer.

  10. Characterizing p -wave superconductivity using the spin structure of Shiba states

    NASA Astrophysics Data System (ADS)

    Kaladzhyan, V.; Bena, C.; Simon, P.

    2016-06-01

    Cooper pairs in two-dimensional unconventional superconductors with broken inversion symmetry are in a mixture of an even-parity spin-singlet pairing state with an odd-parity spin-triplet pairing state. We study the magnetic properties of the impurity bound states in such superconductors and find striking signatures in their spin polarization which allow one to unambiguously discriminate a nontopological superconducting phase from a topological one. Moreover, we show how these properties, which could be measured using spin-polarized scanning tunneling microscopy (STM), also enable one to determine the direction of the spin-triplet pairing vector of the host material and thus to distinguish between different types of unconventional pairing.

  11. Universal scaling for the spin-electricity conversion on surface states of topological insulators

    NASA Astrophysics Data System (ADS)

    Yamamoto, K. T.; Shiomi, Y.; Segawa, Kouji; Ando, Yoichi; Saitoh, E.

    2016-07-01

    We have investigated spin-electricity conversion on surface states of bulk-insulating topological insulator (TI) materials using a spin-pumping technique. The sample structure is Ni-Fe ∣Cu ∣TI trilayers, in which magnetic proximity effects on the TI surfaces are negligibly small owing to the inserted Cu layer. Voltage signals produced by the spin-electricity conversion are clearly observed and are enhanced with decreasing temperature, in line with the dominant surface transport at lower temperatures. The efficiency of the spin-electricity conversion is greater for TI samples with a higher resistivity of bulk states and longer mean free path of surface states, consistent with the surface spin-electricity conversion.

  12. A quaternionic map for the steady states of the Heisenberg spin-chain

    NASA Astrophysics Data System (ADS)

    Mehta, Mitaxi P.; Dutta, Souvik; Tiwari, Shubhanshu

    2014-01-01

    We show that the steady states of the classical Heisenberg XXX spin-chain in an external magnetic field can be found by iterations of a quaternionic map. A restricted model, e.g., the xy spin-chain is known to have spatially chaotic steady states and the phase space occupied by these chaotic states is known to go through discrete changes as the field strength is varied. The same phenomenon is studied for the xxx spin-chain. It is seen that in this model the phase space volume varies smoothly with the external field.

  13. Proposal for the creation and optical detection of spin cat states in Bose-Einstein condensates.

    PubMed

    Lau, Hon Wai; Dutton, Zachary; Wang, Tian; Simon, Christoph

    2014-08-29

    We propose a method to create "spin cat states," i.e., macroscopic superpositions of coherent spin states, in Bose-Einstein condensates using the Kerr nonlinearity due to atomic collisions. Based on a detailed study of atom loss, we conclude that cat sizes of hundreds of atoms should be realistic. The existence of the spin cat states can be demonstrated by optical readout. Our analysis also includes the effects of higher-order nonlinearities, atom number fluctuations, and limited readout efficiency. PMID:25215963

  14. Magnetoresistance in the Spin-Orbit Kondo State of Elemental Bismuth

    PubMed Central

    Craco, Luis; Leoni, Stefano

    2015-01-01

    Materials with strong spin-orbit coupling, which competes with other particle-particle interactions and external perturbations, offer a promising route to explore novel phases of quantum matter. Using LDA + DMFT we reveal the complex interplay between local, multi-orbital Coulomb and spin-orbit interaction in elemental bismuth. Our theory quantifies the role played by collective dynamical fluctuations in the spin-orbit Kondo state. The correlated electronic structure we derive is promising in the sense that it leads to results that might explain why moderate magnetic fields can generate Dirac valleys and directional-selective magnetoresistance responses within spin-orbit Kondo metals. PMID:26358556

  15. Direct measurement of nonlocal entanglement of two-qubit spin quantum states.

    PubMed

    Cheng, Liu-Yong; Yang, Guo-Hui; Guo, Qi; Wang, Hong-Fu; Zhang, Shou

    2016-01-01

    We propose efficient schemes of direct concurrence measurement for two-qubit spin and photon-polarization entangled states via the interaction between single-photon pulses and nitrogen-vacancy (NV) centers in diamond embedded in optical microcavities. For different entangled-state types, diversified quantum devices and operations are designed accordingly. The initial unknown entangled states are possessed by two spatially separated participants, and nonlocal spin (polarization) entanglement can be measured with the aid of detection probabilities of photon (NV center) states. This non-demolition entanglement measurement manner makes initial entangled particle-pair avoid complete annihilation but evolve into corresponding maximally entangled states. Moreover, joint inter-qubit operation or global qubit readout is not required for the presented schemes and the final analyses inform favorable performance under the current parameters conditions in laboratory. The unique advantages of spin qubits assure our schemes wide potential applications in spin-based solid quantum information and computation. PMID:26778340

  16. Direct measurement of nonlocal entanglement of two-qubit spin quantum states

    NASA Astrophysics Data System (ADS)

    Cheng, Liu-Yong; Yang, Guo-Hui; Guo, Qi; Wang, Hong-Fu; Zhang, Shou

    2016-01-01

    We propose efficient schemes of direct concurrence measurement for two-qubit spin and photon-polarization entangled states via the interaction between single-photon pulses and nitrogen-vacancy (NV) centers in diamond embedded in optical microcavities. For different entangled-state types, diversified quantum devices and operations are designed accordingly. The initial unknown entangled states are possessed by two spatially separated participants, and nonlocal spin (polarization) entanglement can be measured with the aid of detection probabilities of photon (NV center) states. This non-demolition entanglement measurement manner makes initial entangled particle-pair avoid complete annihilation but evolve into corresponding maximally entangled states. Moreover, joint inter-qubit operation or global qubit readout is not required for the presented schemes and the final analyses inform favorable performance under the current parameters conditions in laboratory. The unique advantages of spin qubits assure our schemes wide potential applications in spin-based solid quantum information and computation.

  17. Direct measurement of nonlocal entanglement of two-qubit spin quantum states

    PubMed Central

    Cheng, Liu-Yong; Yang, Guo-Hui; Guo, Qi; Wang, Hong-Fu; Zhang, Shou

    2016-01-01

    We propose efficient schemes of direct concurrence measurement for two-qubit spin and photon-polarization entangled states via the interaction between single-photon pulses and nitrogen-vacancy (NV) centers in diamond embedded in optical microcavities. For different entangled-state types, diversified quantum devices and operations are designed accordingly. The initial unknown entangled states are possessed by two spatially separated participants, and nonlocal spin (polarization) entanglement can be measured with the aid of detection probabilities of photon (NV center) states. This non-demolition entanglement measurement manner makes initial entangled particle-pair avoid complete annihilation but evolve into corresponding maximally entangled states. Moreover, joint inter-qubit operation or global qubit readout is not required for the presented schemes and the final analyses inform favorable performance under the current parameters conditions in laboratory. The unique advantages of spin qubits assure our schemes wide potential applications in spin-based solid quantum information and computation. PMID:26778340

  18. Criterion and flexibility of operation difficulty for perfect teleportation of arbitrary n-qutrit state with ( n: n)-qutrit pure state

    NASA Astrophysics Data System (ADS)

    Zhang, ZiYun; Liu, YiMin; Zhang, Wen; Zhang, ZhanJun

    2011-08-01

    Under the preconditions that a ( n: n)-qutrit pure state is taken as the quantum channel to teleport an arbitrary n-qutrit state and the sender is able to perform generalized-Bell-state measurements and publish the results, the necessary transformation operation in the receiver's site is worked out in terms of the technique of swapping states. A criterion on whether such quantum channel can be utilized for perfect teleportation is derived by virtue of the unitarity of the resultant transformation operator. Moreover, the flexibility between the measurement difficulty and the reconstruction difficulty is shown and discussed.

  19. The spin state of iron in minerals of Earth's lower mantle

    DOE PAGESBeta

    Sturhahn, Wolfgang; Jackson, Jennifer M.; Lin, Jung -Fu

    2005-06-23

    Here, the spin state of Fe(II) and Fe(III) at temperatures and pressures typical for the Earth's lower mantle is discussed. We predict an extended high-spin to low-spin crossover region along the geotherm for Fe-dilute systems depending on crystal-field splitting, pairing energy, and cooperative interactions. In particular, spin transitions in ferromagnesium silicate perovskite and ferropericlase, the dominant lower mantle components, should occur in a wide temperature-pressure range. We also derive a gradual volume change associated with such transitions in the lower mantle. The gradual density changes and the wide spin crossover regions seem incompatible with lower mantle stratification resulting from amore » spin transition.« less

  20. Critical competition between two distinct orbital-spin ordered states in perovskite vanadates

    NASA Astrophysics Data System (ADS)

    Fujioka, J.; Yasue, T.; Miyasaka, S.; Yamasaki, Y.; Arima, T.; Sagayama, H.; Inami, T.; Ishii, K.; Tokura, Y.

    2010-10-01

    We have investigated the spin/orbital phase diagram in the perovskite orthovanadate RVO3 ( R=Eu , Y, Dy, and Ho) by measurements of magnetization, dielectric constant, specific heat, Raman scattering spectra, and x-ray diffraction, focusing on the interplay between the V3d spin and the 4f moment of the R ion. The thermally induced phase transition between the C-type spin/G-type orbital ordered state and the G-type spin/C-type orbital ordered state is observed for Eu1-xYxVO3 (x=0-0.52) without 4f moment. By comparing this phase diagram with the spin/orbital ordering in TbVO3 , it is evident that the critical competition between the C-type spin/G-type orbital ordered phase and the G-type spin/C-type orbital ordered one depends not only on the GdFeO3 -type lattice distortion but also on the presence of the 4f moment of the R ion. The magnetic field induced phase transition of the spin/orbital ordering is achieved concomitantly with polarizing R4f moments for DyVO3 and HoVO3 . For DyVO3 , the G-type spin/C-type orbital ordered phase is switched to the C-type spin/G-type orbital ordered one by applying a moderate magnetic field around 3 T. By contrast, the G-type spin/C-type orbital ordering is rather favored under the magnetic field in HoVO3 . The results cannot be uniquely explained in terms of the exchange interaction between the V3d spin and the R -ion 4f moment. The coupling of the R4f moment polarization with the lattice distortion tied with the orbital ordering of the V3d sublattice may also be relevant to this field induced phase transition.

  1. Quantum filter of spin polarized states: Metal–dielectric–ferromagnetic/semiconductor device

    SciTech Connect

    Makarov, Vladimir I.; Khmelinskii, Igor

    2014-02-01

    Highlights: • Development of a new spintronics device. • Development of quantum spin polarized filters. • Development of theory of quantum spin polarized filter. - Abstract: Recently we proposed a model for the Quantum Spin-Polarized State Filter (QSPSF). The magnetic moments are transported selectively in this model, detached from the electric charge carriers. Thus, transfer of a spin-polarized state between two conductors was predicted in a system of two levels coupled by exchange interaction. The strength of the exchange interaction between the two conductive layers depends on the thickness of the dielectric layer separating them. External magnetic fields modulate spin-polarized state transfer, due to Zeeman level shift. Therefore, a linearly growing magnetic field generates a series of current peaks in a nearby coil. Thus, our spin-state filter should contain as least three nanolayers: (1) conductive or ferromagnetic; (2) dielectric; and (3) conductive or semiconductive. The spectrum of spin-polarized states generated by the filter device consists of a series of resonance peaks. In a simple case the number of lines equals S, the total spin angular momentum of discrete states in one of the coupled nanolayers. Presently we report spin-polarized state transport in metal–dielectric–ferromagnetic (MDF) and metal–dielectric–semiconductor (MDS) three-layer sandwich devices. The exchange-resonance spectra in such devices are quite specific, differing also from spectra observed earlier in other three-layer devices. The theoretical model is used to interpret the available experimental results. A detailed ab initio analysis of the magnetic-field dependence of the output magnetic moment averaged over the surface of the device was carried out. The model predicts the resonance structure of the signal, although at its present accuracy it cannot predict the positions of the spectral peaks.

  2. Spin-state blockade in Te6+-substituted electron-doped LaCoO3

    NASA Astrophysics Data System (ADS)

    Tomiyasu, Keisuke; Koyama, Shun-Ichi; Watahiki, Masanori; Sato, Mika; Nishihara, Kazuki; Onodera, Mitsugi; Iwasa, Kazuaki; Nojima, Tsutomu; Yamasaki, Yuuichi; Nakao, Hironori; Murakami, Youichi

    2015-03-01

    Perovskite-type LaCoO3 (Co3+: d6) is a rare inorganic material with sensitive and characteristic responses among low, intermediate, and high spin states. For example, in insulating nonmagnetic low-spin states below about 20 K, light hole doping (Ni substitution) induces much larger magnetization than expected; over net 10μB/hole (5μB/Ni) for 1μB/hole (1μB/Ni), in which the nearly isolated dopants locally change the surrounding Co low-spin states to magnetic ones and form spin molecules with larger total spin. Further, the former is isotropic, whereas the latter exhibits characteristic anisotropy probably because of Jahn-Teller distortion. In contrast, for electron doping, relatively insensitive spin-state responses were reported, as in LaCo(Ti4+) O3, but are not clarified, and are somewhat controversial. Here, we present macroscopic measurement data of another electron-doped system LaCo(Te6+) O3 and discuss the spin-state responses. This study was financially supported by Grants-in-Aid for Young Scientists (B) (No. 22740209 and 26800174) from the MEXT of Japan.

  3. High-fidelity projective read-out of a solid-state spin quantum register.

    PubMed

    Robledo, Lucio; Childress, Lilian; Bernien, Hannes; Hensen, Bas; Alkemade, Paul F A; Hanson, Ronald

    2011-09-29

    Initialization and read-out of coupled quantum systems are essential ingredients for the implementation of quantum algorithms. Single-shot read-out of the state of a multi-quantum-bit (multi-qubit) register would allow direct investigation of quantum correlations (entanglement), and would give access to further key resources such as quantum error correction and deterministic quantum teleportation. Although spins in solids are attractive candidates for scalable quantum information processing, their single-shot detection has been achieved only for isolated qubits. Here we demonstrate the preparation and measurement of a multi-spin quantum register in a low-temperature solid-state system by implementing resonant optical excitation techniques originally developed in atomic physics. We achieve high-fidelity read-out of the electronic spin associated with a single nitrogen-vacancy centre in diamond, and use this read-out to project up to three nearby nuclear spin qubits onto a well-defined state. Conversely, we can distinguish the state of the nuclear spins in a single shot by mapping it onto, and subsequently measuring, the electronic spin. Finally, we show compatibility with qubit control: we demonstrate initialization, coherent manipulation and single-shot read-out in a single experiment on a two-qubit register, using techniques suitable for extension to larger registers. These results pave the way for a test of Bell's inequalities on solid-state spins and the implementation of measurement-based quantum information protocols. PMID:21937989

  4. Mechanism of dilute-spin-exchange in solid-state NMR

    SciTech Connect

    Lu, George J.; Opella, Stanley J.

    2014-03-28

    In the stationary, aligned samples used in oriented sample (OS) solid-state NMR, {sup 1}H-{sup 1}H homonuclear dipolar couplings are not attenuated as they are in magic angle spinning solid-state NMR; consequently, they are available for participation in dipolar coupling-based spin-exchange processes. Here we describe analytically the pathways of {sup 15}N-{sup 15}N spin-exchange mediated by {sup 1}H-{sup 1}H homonuclear dipolar couplings. The mixed-order proton-relay mechanism can be differentiated from the third spin assisted recoupling mechanism by setting the {sup 1}H to an off-resonance frequency so that it is at the “magic angle” during the spin-exchange interval in the experiment, since the “magic angle” irradiation nearly quenches the former but only slightly attenuates the latter. Experimental spectra from a single crystal of N-acetyl leucine confirm that this proton-relay mechanism plays the dominant role in {sup 15}N-{sup 15}N dilute-spin-exchange in OS solid-state NMR in crystalline samples. Remarkably, the “forbidden” spin-exchange condition under “magic angle” irradiation results in {sup 15}N-{sup 15}N cross-peaks intensities that are comparable to those observed with on-resonance irradiation in applications to proteins. The mechanism of the proton relay in dilute-spin-exchange is crucial for the design of polarization transfer experiments.

  5. Improved spin squeezing of an atomic ensemble through internal state control

    NASA Astrophysics Data System (ADS)

    Hemmer, Daniel; Montano, Enrique; Deutsch, Ivan; Jessen, Poul

    2016-05-01

    Squeezing of collective atomic spins is typically generated by quantum backaction from a QND measurement of the relevant spin component. In this scenario the degree of squeezing is determined by the measurement resolution relative to the quantum projection noise (QPN) of a spin coherent state (SCS). Greater squeezing can be achieved through optimization of the 3D geometry of probe and atom cloud, or by placing the atoms in an optical cavity. We explore here a complementary strategy that relies on quantum control of the large internal spin available in alkali atoms such as Cs. Using a combination of rf and uw magnetic fields, we coherently map the internal spins in our ensemble from the SCS (| f = 4, m = 4>) to a ``cat'' state which is an equal superposition of | f = 4, m = 4>and | f = 4, m = -4>. This increases QPN by a factor of 2 f = 8 relative to the SCS, and therefore the amount of backaction and spin-spin entanglement produced by our QND measurement. In a final step, squeezing generated in the cat state basis can be mapped back to the SCS basis, where it corresponds to increased squeezing of the physical spin. Our experiments suggest that up to 8dB of metrologically useful squeezing can be generated in this way, compared to ~ 3 dB in an otherwise identical experiment starting from a SCS.

  6. Quantum model of a solid-state spin qubit: Ni cluster on a silicon surface by the generalized spin Hamiltonian and X-ray absorption spectroscopy investigations

    NASA Astrophysics Data System (ADS)

    Farberovich, Oleg V.; Mazalova, Victoria L.; Soldatov, Alexander V.

    2015-11-01

    We present here the quantum model of a Ni solid-state electron spin qubit on a silicon surface with the use of a density-functional scheme for the calculation of the exchange integrals in the non-collinear spin configurations in the generalized spin Hamiltonian (GSH) with the anisotropic exchange coupling parameters linking the nickel ions with a silicon substrate. In this model the interaction of a spin qubit with substrate is considered in GSH at the calculation of exchange integrals Jij of the nanosystem Ni7-Si in the one-electron approach taking into account chemical bonds of all Si-atoms of a substrate (environment) with atoms of the Ni7-cluster. The energy pattern was found from the effective GSH Hamiltonian acting in the restricted spin space of the Ni ions by the application of the irreducible tensor operators (ITO) technique. In this paper we offer the model of the quantum solid-state N-spin qubit based on the studying of the spin structure and the spin-dynamics simulations of the 3d-metal Ni clusters on the silicon surface. The solution of the problem of the entanglement between spin states in the N-spin systems is becoming more interesting when considering clusters or molecules with a spectral gap in their density of states. For quantifying the distribution of the entanglement between the individual spin eigenvalues (modes) in the spin structure of the N-spin system we use the density of entanglement (DOE). In this study we have developed and used the advanced high-precision numerical techniques to accurately assess the details of the decoherence process governing the dynamics of the N-spin qubits interacting with a silicon surface. We have studied the Rabi oscillations to evaluate the N-spin qubits system as a function of the time and the magnetic field. We have observed the stabilized Rabi oscillations and have stabilized the quantum dynamical qubit state and Rabi driving after a fixed time (0.327 μs). The comparison of the energy pattern with the

  7. Quantum nonlocality of generic family of four-qubit entangled pure states

    NASA Astrophysics Data System (ADS)

    Ding, Dong; He, Ying-Qiu; Yan, Feng-Li; Gao, Ting

    2015-07-01

    We directly introduce a Bell-type inequality for four-qubit systems. Using the inequality we investigate quantum nonlocality of a generic family of states |Gabcd> [Phys. Rev. A 65 052112 (2002)] and several canonical four-qubit entangled states. It has been demonstrated that the inequality is maximally violated by the so called “four-qubit the maximally entangled state |Gm>” and it is also violated by four-qubit W state and a special family of states |Gab00>. Moreover, a useful entanglement-nonlocality relationship for the family of states |Gab00> is derived. Finally, we present a scheme of preparation of the state |Gm> with linear optics and cross-Kerr nonlinearities. Project supported by the National Natural Science Foundation of China (Grant Nos. 11475054 and 11371005), Hebei Natural Science Foundation of China (Grant Nos. A2012205013 and A2014205060), the Fundamental Research Funds for the Central Universities of Ministry of Education of China (Grant Nos. 3142014068 and 3142014125), and Langfang Key Technology Research and Development Program of China (Grant No. 2014011002).

  8. New high spin states and isomers in the {sup 208}Pb and {sup 207}Pb nuclei

    SciTech Connect

    Broda, R.; Wrzesinski, J.; Pawlat, T.

    1996-12-31

    The two most prominent examples of the heavy doubly closed shell (DCS) nuclei, {sup 208}Pb and {sup 132}Sn, are not accessible by conventional heavy-ion fusion processes populating high-spin states. This experimental difficulty obscured for a long time the investigation of yrast high-spin states in both DCS and neighboring nuclei and consequently restricted the study of the shell model in its most attractive regions. Recent technical development of multidetector gamma arrays opened new ways to exploit more complex nuclear processes which populate the nuclei of interest with suitable yields for gamma spectroscopy and involve population of moderately high spin states. This new possibility extended the range of accessible spin values and is a promising way to reach new yrast states. Some of these states are expected to be of high configurational purity and can be a source of important shell model parameters which possibly can be used later to check the validity of the spherical shell model description at yet higher spin and higher excitation energy. The nuclei in the closest vicinity of {sup 132}Sn are produced in spontaneous fission and states with spin values up to I=14 can be reached in fission gamma spectroscopy studies with the presently achieved sensitivity of gamma arrays. New results on yrast states in the {sup 134}Te and {sup 135}I nuclei populated in fission of the {sup 248}Cm presented at this conference illustrate such application of the resolving power offered by modern gamma techniques.

  9. Universal scheme for finite-probability perfect transfer of arbitrary multispin states through spin chains

    SciTech Connect

    Man, Zhong-Xiao; An, Nguyen Ba; Xia, Yun-Jie; Kim, Jaewan

    2014-12-15

    In combination with the theories of open system and quantum recovering measurement, we propose a quantum state transfer scheme using spin chains by performing two sequential operations: a projective measurement on the spins of ‘environment’ followed by suitably designed quantum recovering measurements on the spins of interest. The scheme allows perfect transfer of arbitrary multispin states through multiple parallel spin chains with finite probability. Our scheme is universal in the sense that it is state-independent and applicable to any model possessing spin–spin interactions. We also present possible methods to implement the required measurements taking into account the current experimental technologies. As applications, we consider two typical models for which the probabilities of perfect state transfer are found to be reasonably high at optimally chosen moments during the time evolution. - Highlights: • Scheme that can achieve perfect quantum state transfer is devised. • The scheme is state-independent and applicable to any spin-interaction models. • The scheme allows perfect transfer of arbitrary multispin states. • Applications to two typical models are considered in detail.

  10. Quantum-teleportation benchmarks for independent and identically distributed spin states and displaced thermal states

    SciTech Connect

    Guta, Madalin; Bowles, Peter; Adesso, Gerardo

    2010-10-15

    A successful state-transfer (or teleportation) experiment must perform better than the benchmark set by the 'best' measure and prepare procedure. We consider the benchmark problem for the following families of states: (i) displaced thermal equilibrium states of a given temperature; (ii) independent identically prepared qubits with a completely unknown state. For the first family we show that the optimal procedure is heterodyne measurement followed by the preparation of a coherent state. This procedure was known to be optimal for coherent states and for squeezed states with the 'overlap fidelity' as the figure of merit. Here, we prove its optimality with respect to the trace norm distance and supremum risk. For the second problem we consider n independent and identically distributed (i.i.d.) spin-(1/2) systems in an arbitrary unknown state {rho} and look for the measurement-preparation pair (M{sub n},P{sub n}) for which the reconstructed state {omega}{sub n}:=P{sub n} circle M{sub n}({rho}{sup xn}) is as close as possible to the input state (i.e., parallel {omega}{sub n}-{rho}{sup xn} parallel {sub 1} is small). The figure of merit is based on the trace norm distance between the input and output states. We show that asymptotically with n this problem is equivalent to the first one. The proof and construction of (M{sub n},P{sub n}) uses the theory of local asymptotic normality developed for state estimation which shows that i.i.d. quantum models can be approximated in a strong sense by quantum Gaussian models. The measurement part is identical to 'optimal estimation', showing that 'benchmarking' and estimation are closely related problems in the asymptotic set up.

  11. Spin texture of time-reversal symmetry invariant surface states on W(110)

    PubMed Central

    Kutnyakhov, D.; Chernov, S.; Medjanik, K.; Wallauer, R.; Tusche, C.; Ellguth, M.; Nepijko, S. A.; Krivenkov, M.; Braun, J.; Borek, S.; Minár, J.; Ebert, H.; Elmers, H. J.; Schönhense, G.

    2016-01-01

    We find in the case of W(110) previously overlooked anomalous surface states having their spin locked at right angle to their momentum using spin-resolved momentum microscopy. In addition to the well known Dirac-like surface state with Rashba spin texture near the -point, we observe a tilted Dirac cone with circularly shaped cross section and a Dirac crossing at 0.28 ×   within the projected bulk band gap of tungsten. This state has eye-catching similarities to the spin-locked surface state of a topological insulator. The experiments are fortified by a one-step photoemission calculation in its density-matrix formulation. PMID:27406652

  12. Spin texture of time-reversal symmetry invariant surface states on W(110).

    PubMed

    Kutnyakhov, D; Chernov, S; Medjanik, K; Wallauer, R; Tusche, C; Ellguth, M; Nepijko, S A; Krivenkov, M; Braun, J; Borek, S; Minár, J; Ebert, H; Elmers, H J; Schönhense, G

    2016-01-01

    We find in the case of W(110) previously overlooked anomalous surface states having their spin locked at right angle to their momentum using spin-resolved momentum microscopy. In addition to the well known Dirac-like surface state with Rashba spin texture near the -point, we observe a tilted Dirac cone with circularly shaped cross section and a Dirac crossing at 0.28 ×   within the projected bulk band gap of tungsten. This state has eye-catching similarities to the spin-locked surface state of a topological insulator. The experiments are fortified by a one-step photoemission calculation in its density-matrix formulation. PMID:27406652

  13. Spin texture of time-reversal symmetry invariant surface states on W(110)

    NASA Astrophysics Data System (ADS)

    Kutnyakhov, D.; Chernov, S.; Medjanik, K.; Wallauer, R.; Tusche, C.; Ellguth, M.; Nepijko, S. A.; Krivenkov, M.; Braun, J.; Borek, S.; Minár, J.; Ebert, H.; Elmers, H. J.; Schönhense, G.

    2016-07-01

    We find in the case of W(110) previously overlooked anomalous surface states having their spin locked at right angle to their momentum using spin-resolved momentum microscopy. In addition to the well known Dirac-like surface state with Rashba spin texture near the -point, we observe a tilted Dirac cone with circularly shaped cross section and a Dirac crossing at 0.28 ×   within the projected bulk band gap of tungsten. This state has eye-catching similarities to the spin-locked surface state of a topological insulator. The experiments are fortified by a one-step photoemission calculation in its density-matrix formulation.

  14. High-spin states in the five-valence-particle nucleus {sup 213}Po

    SciTech Connect

    Astier, Alain; Porquet, Marie-Genevieve

    2011-03-15

    Excited states in {sup 213}Po have been populated using the {sup 18}O+ {sup 208}Pb reaction at 85 MeV beam energy and studied with the Euroball IV {gamma} multidetector array. The level scheme has been built up to {approx}2.0 MeV excitation energy and spin I{approx}25/2({h_bar}/2{pi}) from the triple {gamma} coincidence data. Spin and parity values of several yrast states have been assigned from the {gamma} angular properties. The configurations of the yrast states are discussed using results of empirical shell-model calculations and by analogy with the neighboring nuclei. The spin and parity values of several low-spin states of {sup 213}Po previously identified from the {beta} decay of {sup 213}Bi are revised.

  15. Adsorption and spin state properties of Cr, Ni, Mo, and Pt deposited on Li⁺ and Na⁺ monovalent cation impurities of MgO (001) surface: DFT calculations.

    PubMed

    Shalabi, Ahmad S; Assem, Mervat M; Soliman, Kamal A

    2011-12-01

    We have analyzed, by means of density functional theory calculations and the embedded cluster model, the adsorption and spin-state properties of Cr, Ni, Mo, and Pt deposited on a MgO crystal. We considered deposition at the Mg(2+) site of a defect-free surface and at Li(+) and Na(+) sites of impurity-containing surfaces. To avoid artificial polarization effects, clusters of moderate sizes with no border anions were embedded in simulated Coulomb fields that closely approximate the Madelung fields of the host surfaces. The interaction between a transition metal atom and a surface results from a competition between Hund's rule for the adsorbed atom and the formation of a chemical bond at the interface. We found that the adsorption energies of the metal atoms are significantly enhanced by the cation impurities, and the adsorption energies of the low-spin states of spin-quenched complexes are always more favorable than those of the high-spin states. Spin polarization effects tend to preserve the spin states of the adsorbed atoms relative to those of the isolated atoms. The metal-support interactions stabilize the low-spin states of the adsorbed metals with respect to the isolated metals, but the effect is not always enough to quench the spin. Spin quenching occurs for Cr and Mo complexes at the Mg(2+) site of the pure surface and at Li(+) and Na(+) sites of the impurity-containing surfaces. Variations of the spin-state properties of free metals and of the adsorption and spin-state properties of metal complexes are correlated with the energies of the frontier orbitals. The electrostatic potential energy curves provide further understanding of the nature of the examined properties. PMID:21369929

  16. Muon Spin Relaxation Evidence for the U(1) Quantum Spin-Liquid Ground State in the Triangular Antiferromagnet YbMgGaO_{4}.

    PubMed

    Li, Yuesheng; Adroja, Devashibhai; Biswas, Pabitra K; Baker, Peter J; Zhang, Qian; Liu, Juanjuan; Tsirlin, Alexander A; Gegenwart, Philipp; Zhang, Qingming

    2016-08-26

    Muon spin relaxation (μSR) experiments on single crystals of the structurally perfect triangular antiferromagnet YbMgGaO_{4} indicate the absence of both static long-range magnetic order and spin freezing down to 0.048 K in a zero field. Below 0.4 K, the μ^{+} spin relaxation rates, which are proportional to the dynamic correlation function of the Yb^{3+} spins, exhibit temperature-independent plateaus. All these μSR results unequivocally support the formation of a gapless U(1) quantum spin liquid ground state in the triangular antiferromagnet YbMgGaO_{4}. PMID:27610879

  17. Frozen Spin Ice Ground States in the Pyrochlore Magnet Tb2Ti2O7

    NASA Astrophysics Data System (ADS)

    Fritsch, Katharina

    2015-03-01

    The ground state nature of the candidate spin liquid pyrochlore magnet Tb2Ti2O7 has remained a puzzle for over 15 years. Despite theoretical expectations of magnetic order below ~ 1 K based on classical Ising-like Tb 3 + spins, early μSR and neutron scattering experiments showed no long range order down to 50 mK. This motivated two theoretical scenarios to account for the apparently disordered ground state: a quantum spin ice scenario in which the classical spin order is suppressed by virtual crystal field excitations that renormalize the antiferromagnetic exchange, or a scenario arising from a yet to be observed structural distortion creating a non-magnetic singlet ground state. I will discuss our time-of-flight neutron scattering measurements on Tb2Ti2O7 that reveal a glassy spin ice ground state, characterized by frozen antiferromagnetic short range order and the formation of a ~ 0.08 meV energy gap in its spin excitation spectrum at the (1/2,1/2,1/2) quasi-ordering wave vectors. A new H - T phase diagram for Tb2Ti2O7 in [110] magnetic field will be presented. I will further discuss recent experiments on slightly off-stoichiometric Tb2+xTi2-xO7-y samples, which also display the same gapped spin ice correlations at (1/2,1/2,1/2) wave vectors.

  18. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves

    SciTech Connect

    Marino, Andrea; Buron-Le Cointe, M.; Lorenc, M.; Toupet, L.; Henning, Robert W.; DiChiara, A. D.; Moffat, Keith

    2015-01-01

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. By combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW

  19. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves

    DOE PAGESBeta

    Marino, Andrea; Buron-Le Cointe, M.; Lorenc, M.; Toupet, L.; Henning, Robert W.; DiChiara, A. D.; Moffat, Keith; Brefuel, N.; Collet, E.

    2015-01-28

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. Lastly, by combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW

  20. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves

    SciTech Connect

    Marino, Andrea; Buron-Le Cointe, M.; Lorenc, M.; Toupet, L.; Henning, Robert W.; DiChiara, A. D.; Moffat, Keith; Brefuel, N.; Collet, E.

    2015-01-28

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. Lastly, by combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW

  1. Out-of-equilibrium dynamics of photoexcited spin-state concentration waves

    PubMed Central

    Marino, A.; Lorenc, M.; Toupet, L.; Henning, R.; DiChiara, A. D.; Moffat, K.; Bréfuel, N.

    2015-01-01

    The spin crossover compound [FeIIH2L2-Me][PF6]2 presents a two-step phase transition. In the intermediate phase, a spin state concentration wave (SSCW) appears resulting from a symmetry breaking (cell doubling) associated with a long-range order of alternating high and low spin molecular states. By combining time-resolved optical and X-ray diffraction measurements on a single crystal, we study how such a system responds to femtosecond laser excitation and we follow in real time the erasing and rewriting of the SSCW. PMID:25627455

  2. Ballistic quantum state transfer in spin chains: General theory for quasi-free models and arbitrary initial states

    NASA Astrophysics Data System (ADS)

    Banchi, Leonardo

    2013-11-01

    Ballistic quantum information transfer through spin chains is based on the idea of making the spin dynamics ruled by collective excitations with linear dispersion relation. Unlike perfect state transfer schemes, a ballistic transmission requires only a minimal engineering of the interactions; in fact, for most practical purposes, the optimization of the couplings to the ends of the chain is sufficient to obtain an almost perfect transmission. In this work we review different ballistic quantum state transfer protocols based on the dynamics of quasi-free spin chains, and further generalize them both at zero and finite temperature. In particular, besides presenting novel analytical results for XX, XY, and Ising spin models, it is shown how, via a complete control on the first and last two qubits of the chain, destructive thermal effects can be cancelled, leading to a high-quality state transmission irrespective of the temperature.

  3. Conservation of the pure adiabatic state in Ehrenfest dynamics of the photoisomerization of molecules.

    PubMed

    Miyamoto, Yoshiyuki; Tateyama, Yoshitaka; Oyama, Norihisa; Ohno, Takahisa

    2015-01-01

    We examined real-time-propagation time-dependent density functional theory (rtp-TDDFT) coupled with molecular dynamics (MD), which uses single-particle representation of time-evolving wavefunctions allowing exchange of orbital characteristics between occupied and empty states making the effective Kohn-Sham Hamiltonian dependent on the potential energy surfaces (PESs). This scheme is expected to lead to mean-field average of adiabatic potential energy surfaces (PESs), and is one of Ehrenfest (mean-field) approaches. However, we demonstrate that the mean-field average can be absent in simulating photoisomerization of azobenzene and ethylene molecules. A transition from the S2 to the S1 excited state without the mean- field average was observed after examining several rtp-TDDFT-MD trajectories of a photoexcited azobenzene molecule. The subsequent trans-cis isomerization was observed in our simulation, which is consistent with experimental observation and supported by previous calculations. The absence of the mean-field average of PESs was also observed for the transition between the S1 and S0 states, indicating that the MD simulation was on a single PES. Conversely, we found no transition to the ground state (S0 state) when we performed a MD simulation of an S1 excited ethylene molecule owing to the constraint on the occupation number of each molecular orbital. Thus, we conclude that, at least for azobenzene and ethylene molecules, the rtp-TDDFT-MD is an on-the-fly simulation that can automatically see the transition among the PESs of excited states without the mean-field average unless the simulation reaches the PES of the S0 state. PMID:26658633

  4. Conservation of the pure adiabatic state in Ehrenfest dynamics of the photoisomerization of molecules

    PubMed Central

    Miyamoto, Yoshiyuki; Tateyama, Yoshitaka; Oyama, Norihisa; Ohno, Takahisa

    2015-01-01

    We examined real-time-propagation time-dependent density functional theory (rtp-TDDFT) coupled with molecular dynamics (MD), which uses single-particle representation of time-evolving wavefunctions allowing exchange of orbital characteristics between occupied and empty states making the effective Kohn-Sham Hamiltonian dependent on the potential energy surfaces (PESs). This scheme is expected to lead to mean-field average of adiabatic potential energy surfaces (PESs), and is one of Ehrenfest (mean-field) approaches. However, we demonstrate that the mean-field average can be absent in simulating photoisomerization of azobenzene and ethylene molecules. A transition from the S2 to the S1 excited state without the mean- field average was observed after examining several rtp-TDDFT-MD trajectories of a photoexcited azobenzene molecule. The subsequent trans-cis isomerization was observed in our simulation, which is consistent with experimental observation and supported by previous calculations. The absence of the mean-field average of PESs was also observed for the transition between the S1 and S0 states, indicating that the MD simulation was on a single PES. Conversely, we found no transition to the ground state (S0 state) when we performed a MD simulation of an S1 excited ethylene molecule owing to the constraint on the occupation number of each molecular orbital. Thus, we conclude that, at least for azobenzene and ethylene molecules, the rtp-TDDFT-MD is an on-the-fly simulation that can automatically see the transition among the PESs of excited states without the mean-field average unless the simulation reaches the PES of the S0 state. PMID:26658633

  5. Ultrafast quantum spin-state switching in the Co-octaethylporphyrin molecular magnet with a terahertz pulsed magnetic field

    NASA Astrophysics Data System (ADS)

    Farberovich, Oleg V.; Mazalova, Victoria L.

    2016-05-01

    Molecular spin crossover switches are the objects of intense theoretical and experimental studies in recent years. This interest is due to the fact that these systems allow one to control their spin state by applying an external photo-, thermo-, piezo-, or magnetic stimuli. The greatest amount of research is currently devoted to the study of the effect of the photoexcitation on the bi-stable states of spin crossover single molecular magnets (SMMs). The main limitation of photo-induced bi-stable states is their short lifetime. In this paper we present the results of a study of the spin dynamics of the Co-octaethylporphyrin (CoOEP) molecule in the Low Spin (LS) state and the High Spin (HS) state induced by applying the magnetic pulse of 36.8 T. We show that the spin switching in case of the HS state of the CoOEP molecule is characterized by a long lifetime and is dependent on the magnitude and duration of the applied field. Thus, after applying an external stimuli the system in the LS state after the spin switching reverts to its ground state, whereas the system in the HS state remains in the excited state for a long time. We found that the temperature dependency of magnetic susceptibility shows an abrupt thermal spin transition between two spin states at 40 K. Here the proposed theoretical approach opens the way to create modern devices for spintronics with the controllable spin switching process.

  6. Entangled rings, matrix product states, and exact solutions of XYZ spin chains

    SciTech Connect

    Asoudeh, Marzieh; Karimipour, Vahid; Sadrolashrafi, Afsaneh

    2007-07-15

    We show that the ground state of the Heisenberg spin-1/2 chain in an external magnetic field, can be exactly expressed as a matrix product state, provided that the coupling constants are constrained to be on a specific two dimensional surface. This ground state has a very interesting property: all the pairs of spins are equally entangled with each other. In this last respect, the results are of interest for engineering long-range entanglement in experimentally realizable finite arrays of qubits, where the ground state will act as the initial state of a quantum computer.

  7. Quantum chemical study of Co3+ spin states in LaCoO3

    NASA Astrophysics Data System (ADS)

    Siurakshina, L.; Paulus, B.; Yushankhai, V.; Sivachenko, E.

    2010-03-01

    Ab initio quantum-chemical cluster calculations are performed for the perovskite LaCoO3. The main concern is to calculate the energy level ordering of different spin states of Co3+, which is an issue of great controversy for many years. The calculations performed for the trigonal lattice structure at T = 5 K and 300 K, with the structural data taken from experiment, display that the low-spin (LS, S = 0) ground state is separated from the first excited high-spin (HS, S = 2) state by a gap <100 meV, while the intermediate-spin (IS, S = 1) state is located at much higher energy ≈0.5 eV. We suggest that the local lattice relaxation around the Co3+ ion excited to the HS state and the spin-orbit coupling reduce the spin gap to a value 10 meV. Coupling of the IS state to the Jahn-Teller local lattice distortion is found to be rather strong and reduces its energy position to a value of 200 div 300 meV. Details of the quantum-chemical cluster calculation procedure and the obtained results are extensively discussed and compared with those reported earlier by other authors.

  8. TRANSIENT AND STEADY STATE STUDY OF PURE AND MIXED REFRIGERANTS IN A RESIDENTIAL HEAT PUMP

    EPA Science Inventory

    The report gives results of an experimental and theoretical investigation of the transient and steady state performance of a residential air-conditioning/heat pump (AC/HP) operating with different refrigerants. (NOTE: The project was motivated by environmental concerns related to...

  9. Existence of an exotic torus configuration in high-spin excited states of 40Ca.

    PubMed

    Ichikawa, T; Maruhn, J A; Itagaki, N; Matsuyanagi, K; Reinhard, P-G; Ohkubo, S

    2012-12-01

    We investigate the possibility of the existence of the exotic torus configuration in the high-spin excited states of (40)Ca. We here consider the spin alignments about the symmetry axis. To this end, we use a three-dimensional cranked Skyrme Hartree-Fock method and search for stable single-particle configurations. We find one stable state with the torus configuration at the total angular momentum J=60 ħ and an excitation energy of about 170 MeV in all calculations using various Skyrme interactions. The total angular momentum J=60 ħ consists of aligned 12 nucleons with the orbital angular momenta Λ=+4, +5, and +6 for spin-up or -down neutrons and protons. The obtained results strongly suggest that a macroscopic amount of circulating current breaking the time-reversal symmetry emerges in the high-spin excited state of (40)Ca. PMID:23368188

  10. Quantum teleportation from a propagating photon to a solid-state spin qubit

    NASA Astrophysics Data System (ADS)

    Gao, W. B.; Fallahi, P.; Togan, E.; Delteil, A.; Chin, Y. S.; Miguel-Sanchez, J.; Imamoğlu, A.

    2013-11-01

    A quantum interface between a propagating photon used to transmit quantum information and a long-lived qubit used for storage is of central interest in quantum information science. A method for implementing such an interface between dissimilar qubits is quantum teleportation. Here we experimentally demonstrate transfer of quantum information carried by a photon to a semiconductor spin using quantum teleportation. In our experiment, a single photon in a superposition state is generated using resonant excitation of a neutral dot. To teleport this photonic qubit, we generate an entangled spin-photon state in a second dot located 5 m away and interfere the photons from the two dots in a Hong-Ou-Mandel set-up. Thanks to an unprecedented degree of photon-indistinguishability, a coincidence detection at the output of the interferometer heralds successful teleportation, which we verify by measuring the resulting spin state after prolonging its coherence time by optical spin-echo.

  11. Role of metastable charge states in a quantum-dot spin-qubit readout

    NASA Astrophysics Data System (ADS)

    Mason, J. D.; Studenikin, S. A.; Kam, A.; Wasilewski, Z. R.; Sachrajda, A. S.; Kycia, J. B.

    2015-09-01

    Readout of a spin qubit in a lateral gate-defined quantum-dot device typically involves a charge detector and a spin-to-charge conversion technique employing spin blockade. We investigate alternative mechanisms for spin-to-charge conversion involving metastable excited charge states made possible by an asymmetry in the tunneling rates to the leads. This technique is used to observe Landau-Zener-Stückelberg oscillations of the S -T+ qubit within the (1,0) ground state region of the charge stability diagram. The oscillations are π phase shifted relative to those detected using the standard technique and display a nonsinusoidal waveform due to the increased relaxation time from the metastable state.

  12. Quantum teleportation from a propagating photon to a solid-state spin qubit.

    PubMed

    Gao, W B; Fallahi, P; Togan, E; Delteil, A; Chin, Y S; Miguel-Sanchez, J; Imamoğlu, A

    2013-01-01

    A quantum interface between a propagating photon used to transmit quantum information and a long-lived qubit used for storage is of central interest in quantum information science. A method for implementing such an interface between dissimilar qubits is quantum teleportation. Here we experimentally demonstrate transfer of quantum information carried by a photon to a semiconductor spin using quantum teleportation. In our experiment, a single photon in a superposition state is generated using resonant excitation of a neutral dot. To teleport this photonic qubit, we generate an entangled spin-photon state in a second dot located 5 m away and interfere the photons from the two dots in a Hong-Ou-Mandel set-up. Thanks to an unprecedented degree of photon-indistinguishability, a coincidence detection at the output of the interferometer heralds successful teleportation, which we verify by measuring the resulting spin state after prolonging its coherence time by optical spin-echo. PMID:24177228

  13. Magnetic field effects and the role of spin states in singlet fission

    NASA Astrophysics Data System (ADS)

    Burdett, Jonathan J.; Piland, Geoffrey B.; Bardeen, Christopher J.

    2013-10-01

    Singlet fission is a photophysical process that has promise for increasing the efficiency of solar cells. The dynamics depend on triplet spin states and can be influenced by external magnetic fields. In 4-electron systems, fission takes an initial singlet state into a superposition of triplet pair states. Direct evidence for this superposition state is provided by quantum beats in the delayed fluorescence of tetracene crystals. The beat frequencies depend on crystal orientation with respect to the magnetic field, consistent with predictions based on solving the full spin Hamiltonian. Magnetic field effects on the kinetics are analyzed in terms of a hybrid quantum-kinetic model. The magnetic field has no effect on the initial fluorescence decay rate but affects the decay after the triplet pair states begin to equilibrate with the singlets. The long-time behavior of the fluorescence decay reflects association and separation of triplet pairs and relaxation into different spin states.

  14. The steady state solutions of radiatively driven stellar winds for a non-Sobolev, pure absorption model

    NASA Technical Reports Server (NTRS)

    Poe, C. H.; Owocki, S. P.; Castor, J. I.

    1990-01-01

    The steady state solution topology for absorption line-driven flows is investigated for the condition that the Sobolev approximation is not used to compute the line force. The solution topology near the sonic point is of the nodal type with two positive slope solutions. The shallower of these slopes applies to reasonable lower boundary conditions and realistic ion thermal speed v(th) and to the Sobolev limit of zero of the usual Castor, Abbott, and Klein model. At finite v(th), this solution consists of a family of very similar solutions converging on the sonic point. It is concluded that a non-Sobolev, absorption line-driven flow with a realistic values of v(th) has no uniquely defined steady state. To the extent that a pure absorption model of the outflow of stellar winds is applicable, radiatively driven winds should be intrinsically variable.

  15. Plug-in Estimator of the Entropy Rate of a Pure-Jump Two-State Markov Process

    NASA Astrophysics Data System (ADS)

    Regnault, Philippe

    2009-12-01

    The entropy of a distribution with finite support is widely used in all applications involving random variables. A natural equivalent for random processes is the entropy rate. For ergodic pure-jump finite-state Markov processes, this rate is an explicit function of the stationary distribution and the infinitesimal generator. The case of two-state Markov processes is of particular interest. We estimate the entropy rate of such processes by plug-in, from estimators of the stationary distribution and the infinitesimal generator. Three situations of observation are discussed, several independant trajectories are observed, one long trajectory is observed, or the process is observed at discrete times. The asymptotic behavior of the plug-in estimators is established.

  16. The proximity of Mercury's spin to Cassini state 1 from adiabatic invariance

    NASA Astrophysics Data System (ADS)

    Peale, S. J.

    2006-04-01

    In determining Mercury's core structure from its rotational properties, the value of the normalized moment of inertia, C/MR, from the location of Cassini 1 is crucial. If Mercury's spin axis occupies Cassini state 1, its position defines the location of the state, where the axis is fixed in the frame precessing with the orbit. Although tidal and core-mantle dissipation drive the spin to the Cassini state with a time scale O(10) years, the spin might still be displaced from the Cassini state if the variations in the orbital elements induced by planetary perturbations, which change the position of the Cassini state, cause the spin to lag behind as it attempts to follow the state. After being brought to the state by dissipative processes, the spin axis is expected to follow the Cassini state for orbit variations with time scales long compared to the 1000 year precession period of the spin about the Cassini state because the solid angle swept out by the spin axis as it precesses is an adiabatic invariant. Short period variations in the orbital elements of small amplitude should cause displacements that are commensurate with the amplitudes of the short period terms. The exception would be if there are forcing terms in the perturbations that are nearly resonant with the 1000 year precession period. The precision of the radar and eventual spacecraft measurements of the position of Mercury's spin axis warrants a check on the likely proximity of the spin axis to the Cassini state. How confident should we be that the spin axis position defines the Cassini state sufficiently well for a precise determination of C/MR? By following simultaneously the spin position and the Cassini state position during long time scale orbital variations over past 3 million years [Quinn, T.R., Tremaine, S., Duncan, M., 1991. Astron. J. 101, 2287-2305] and short time scale variations for 20,000 years [JPL Ephemeris DE 408; Standish, E.M., private communication, 2005], we show that the spin axis

  17. Ising spin network states for loop quantum gravity: a toy model for phase transitions

    NASA Astrophysics Data System (ADS)

    Feller, Alexandre; Livine, Etera R.

    2016-03-01

    Non-perturbative approaches to quantum gravity call for a deep understanding of the emergence of geometry and locality from the quantum state of the gravitational field. Without background geometry, the notion of distance should emerge entirely from the correlations between the gravity fluctuations. In the context of loop quantum gravity, quantum states of geometry are defined as spin networks. These are graphs decorated with spin and intertwiners, which represent quantized excitations of areas and volumes of the space geometry. Here, we develop the condensed-matter point of view on extracting the physical and geometrical information from spin network states: we introduce new Ising spin network states, both in 2d on a square lattice and in 3d on a hexagonal lattice, whose correlations map onto the usual Ising model in statistical physics. We construct these states from the basic holonomy operators of loop gravity and derive a set of local Hamiltonian constraints that entirely characterize our states. We discuss their phase diagram and show how the distance can be reconstructed from the correlations in the various phases. Finally, we propose generalizations of these Ising states, which open the perspective to study the coarse-graining and dynamics of spin network states using well-known condensed-matter techniques and results.

  18. Long-distance entanglement of spin qubits via quantum Hall edge states

    NASA Astrophysics Data System (ADS)

    Yang, Guang; Hsu, Chen-Hsuan; Stano, Peter; Klinovaja, Jelena; Loss, Daniel

    2016-02-01

    The implementation of a functional quantum computer involves entangling and coherent manipulation of a large number of qubits. For qubits based on electron spins confined in quantum dots, which are among the most investigated solid-state qubits at present, architectural challenges are often encountered in the design of quantum circuits attempting to assemble the qubits within the very limited space available. Here, we provide a solution to such challenges based on an approach to realizing entanglement of spin qubits over long distances. We show that long-range Ruderman-Kittel-Kasuya-Yosida interaction of confined electron spins can be established by quantum Hall edge states, leading to an exchange coupling of spin qubits. The coupling is anisotropic and can be either Ising type or XY type, depending on the spin polarization of the edge state. Such a property, combined with the dependence of the electron spin susceptibility on the chirality of the edge state, can be utilized to gain valuable insights into the topological nature of various quantum Hall states.

  19. Long-distance entanglement of spin qubits via quantum Hall edge states

    NASA Astrophysics Data System (ADS)

    Yang, Guang; Hsu, Chen-Hsuan; Stano, Peter; Klinovaja, Jelena; Loss, Daniel

    The implementation of a functional quantum computer involves entangling and coherent manipulation of a large number of qubits. For qubits based on electron spins confined in quantum dots, which are among the most investigated solid-state qubits at present, architectural challenges are often encountered in the design of quantum circuits attempting to assemble the qubits within the very limited space available. Here, we provide a solution to such challenges based on an approach to realizing entanglement of spin qubits over long distances. We show that long-range Ruderman-Kittel-Kasuya-Yosida interaction of confined electron spins can be established by quantum Hall edge states, leading to an exchange coupling of spin qubits. The coupling is anisotropic and can be either Ising-type or XY-type, depending on the spin polarization of the edge state. Such a property, combined with the dependence of the electron-spin susceptibility on the chirality of the edge state, can be utilized to gain valuable insights into the topological nature of various quantum Hall states.

  20. Feedback-stabilization of an arbitrary pure state of a two-level atom

    NASA Astrophysics Data System (ADS)

    Wang, Jin; Wiseman, H. M.

    2001-12-01

    Unit-efficiency homodyne detection of the resonance fluorescence of a two-level atom collapses the quantum state of the atom to a stochastically moving point on the Bloch sphere. Recently, Hofmann, Mahler, and Hess [Phys. Rev. A 57, 4877 (1998)] showed that by making part of the coherent driving proportional to the homodyne photocurrent one can stabilize the state to any point on the bottom-half of the sphere. Here we reanalyze their proposal using the technique of stochastic master equations, allowing their results to be generalized in two ways. First, we show that any point on the upper- or lower-half, but not the equator, of the sphere may be stabilized. Second, we consider nonunit-efficiency detection, and quantify the effectiveness of the feedback by calculating the maximal purity obtainable in any particular direction in Bloch space.

  1. Stress- and pressure-induced iron spin-state crossover in lower mantle minerals

    NASA Astrophysics Data System (ADS)

    Glazyrin, K.; Miyajima, N.; Smith, J.; Lee, K. K.

    2013-12-01

    The spin-state crossover of ferric and ferrous iron is an important feature of major lower mantle minerals, namely magnesium silicate perovskite (Pv) and ferropericlase (Fp). This electronic transition observed in compressed Pv and Fp was initially discovered at ambient temperatures, however it is also expected for the extreme high pressure-high temperature (HP-HT) conditions endemic to planetary interiors, in particular to the Earth's lower mantle. The pressure-induced spin-state crossover of iron in Pv and Fp has been under focus of many studies, however, some aspects have not been explored in great detail. One of these aspects is the influence of non-hydrostatic macro and micro stresses on the spin-state transitions. Hydrostatic pressure is the important thermodynamic property and distinguishing effects of undesirable stresses is important from both a theoretical and experimental point of view. In this work we compress a two-phase polycrystalline mixture containing magnesium silicate Pv (Fe, Al bearing) and Fp. Using high-resolution synchrotron diffraction on laser-heated diamond-anvil cell samples, we explore characteristic signatures for non-hydrostatic stresses and their influence on the spin-state crossover of ferrous and ferric iron in Pv and Fp. We demonstrate how non-hydrostatic stresses affect the starting pressure and width of the ferrous iron spin-state crossover in Fp and compare available literature data with our results with powder and single crystal diffraction data. Finally, we use the dependence of high-spin to low-spin crossover on the ferrous iron concentration in Fp to support a recently predicted gradual decrease of ferrous iron partitioning coefficient value for Pv and Fp under compression. Our results suggest that this change occurs at HP-HT conditions even before the actual spin-state crossover of ferrous iron in Fp.

  2. Repulsively bound exciton-biexciton states in high-spin fermions in optical lattices

    SciTech Connect

    Argueelles, A.; Santos, L.

    2011-03-15

    We show that the interplay between spin-changing collisions and quadratic Zeeman coupling provides a mechanism for the formation of repulsively bound composites in high-spin fermions, which we illustrate by considering spin flips in an initially polarized hard-core one-dimensional Mott insulator of spin-3/2 fermions. We show that after the flips the dynamics is characterized by the creation of two types of exciton-biexciton composites. We analyze the conditions for the existence of these bound states and discuss their intriguing properties. In particular we show that the effective mass and stability of the composites depends nontrivially on spin-changing collisions, on the quadratic Zeeman effect, and on the initial exciton localization. Finally, we show that the composites may remain stable against inelastic collisions, opening the possibility of interesting quantum composite phases.

  3. Spin-orbit coupling controlled ground state in Sr2ScOsO6

    NASA Astrophysics Data System (ADS)

    Taylor, A. E.; Morrow, R.; Fishman, R. S.; Calder, S.; Kolesnikov, A. I.; Lumsden, M. D.; Woodward, P. M.; Christianson, A. D.

    2016-06-01

    We report neutron scattering experiments which reveal a large spin gap in the magnetic excitation spectrum of weakly-monoclinic double perovskite Sr2ScOsO6 . The spin gap is demonstrative of appreciable spin-orbit-induced anisotropy, despite nominally orbitally-quenched 5 d3Os5 + ions. The system is successfully modeled including nearest neighbor interactions in a Heisenberg Hamiltonian with exchange anisotropy. We find that the presence of the spin-orbit-induced anisotropy is essential for the realization of the type I antiferromagnetic ground state. This demonstrates that physics beyond the LS or JJ coupling limits plays an active role in determining the collective properties of 4 d3 and 5 d3 systems and that theoretical treatments must include spin-orbit coupling.

  4. Spin-orbit coupling controlled ground state in Sr2ScOsO6

    DOE PAGESBeta

    Taylor, A. E.; Morrow, R.; Fishman, R. S.; Calder, S.; Kolesnikov, A. I.; Lumsden, M. D.; Woodward, P. M.; Christianson, A. D.

    2016-06-27

    In this paper, we report neutron scattering experiments which reveal a large spin gap in the magnetic excitation spectrum of weakly-monoclinic double perovskite Sr2ScOsO6. The spin gap is demonstrative of appreciable spin-orbit-induced anisotropy, despite nominally orbitally-quenched 5d3Os5+ ions. The system is successfully modeled including nearest neighbor interactions in a Heisenberg Hamiltonian with exchange anisotropy. We find that the presence of the spin-orbit-induced anisotropy is essential for the realization of the type I antiferromagnetic ground state. Finally, this demonstrates that physics beyond the LS or JJ coupling limits plays an active role in determining the collective properties of 4d3 and 5d3more » systems and that theoretical treatments must include spin-orbit coupling.« less

  5. Spin filtering neutrons with a proton target dynamically polarized using photo-excited triplet states

    NASA Astrophysics Data System (ADS)

    Haag, M.; van den Brandt, B.; Eichhorn, T. R.; Hautle, P.; Wenckebach, W. Th.

    2012-06-01

    In a test of principle a neutron spin filter has been built, which is based on dynamic nuclear polarization (DNP) using photo-excited triplet states. This DNP method has advantages over classical concepts as the requirements for cryogenic equipment and magnets are much relaxed: the spin filter is operated in a field of 0.3 T at a temperature of about 100 K and has performed reliably over periods of several weeks. The neutron beam was also used to analyze the polarization of the target employed as a spin filter. We obtained an independent measurement of the proton spin polarization of ˜0.13 in good agreement with the value determined with NMR. Moreover, the neutron beam was used to measure the proton spin polarization as a function of position in the naphthalene sample. The polarization was found to be homogeneous, even at low laser power, in contradiction to existing models describing the photo-excitation process.

  6. Topological quantum phase transitions and edge states in spin-orbital coupled Fermi gases

    PubMed Central

    Zhou, Tao; Gao, Yi; Wang, Z. D.

    2014-01-01

    We study superconducting states in the presence of spin-orbital coupling and Zeeman field. It is found that a phase transition from a Fulde-Ferrell-Larkin-Ovchinnikov state to the topological superconducting state occurs upon increasing the spin-orbital coupling. The nature of this topological phase transition and its critical property are investigated numerically. Physical properties of the topological superconducting phase are also explored. Moreover, the local density of states is calculated, through which the topological feature may be tested experimentally. PMID:24918901

  7. Non-Markovian dynamics of quantum systems. II. Decay rate, capture, and pure states

    SciTech Connect

    Palchikov, Yu.V.; Antonenko, N.V.; Kanokov, Z.; Adamian, G.G.; Scheid, W.

    2005-01-01

    On the basis of a master equation for the reduced density matrix of open quantum systems, we study the influence of time-dependent friction and diffusion coefficients on the decay rate from a potential well and the capture probability into a potential well. Taking into account the mixed diffusion coefficient D{sub qp}, the quasistationary decay rates are compared with the analytically derived Kramers-type formulas for different temperatures and frictions. The diffusion coefficients supplying the purity of states are derived for a non-Markovian dynamics.

  8. Structure determination of individual electron-nuclear spin complexes in a solid-state matrix

    NASA Astrophysics Data System (ADS)

    Laraoui, Abdelghani; Pagliero, Daniela; Meriles, Carlos

    2015-03-01

    A spin-based quantum computer will store and process information via ``spin complexes'' formed by a small number of interacting electronic and nuclear spins within a solid-state host. Unlike present electronic circuits, differences in the atomic composition and local geometry make each of these spin clusters distinct from the rest. Integration of these units into a working network thus builds on our ability to determine the cluster atomic structure, a problem we tackle herein with the aid of a magnetic resonance protocol. Using the nitrogen-vacancy (NV) center in diamond as a model system, we show analytically and numerically that the spatial coordinates of weakly coupled 13C spins can be determined by selectively transferring and retrieving spin polarization. The technique's spatial resolution can reach up to 0.1 nm, limited by the NV spin coherence lifetime. No external magnetic field gradient is required, which makes this imaging scheme applicable to NV-13C complexes buried deep inside the crystal host. Further, this approach can be adapted to nuclear spins other than 13C, and thus applied to the characterization of individual molecules anchored to the diamond surface.

  9. High-fidelity transfer and storage of photon states in a single nuclear spin

    NASA Astrophysics Data System (ADS)

    Yang, Sen; Wang, Ya; Rao, D. D. Bhaktavatsala; Hien Tran, Thai; Momenzadeh, Ali S.; Markham, M.; Twitchen, D. J.; Wang, Ping; Yang, Wen; Stöhr, Rainer; Neumann, Philipp; Kosaka, Hideo; Wrachtrup, Jörg

    2016-08-01

    Long-distance quantum communication requires photons and quantum nodes that comprise qubits for interaction with light and good memory capabilities, as well as processing qubits for the storage and manipulation of photons. Owing to the unavoidable photon losses, robust quantum communication over lossy transmission channels requires quantum repeater networks. A necessary and highly demanding prerequisite for these networks is the existence of quantum memories with long coherence times to reliably store the incident photon states. Here we demonstrate the high-fidelity (∼98%) coherent transfer of a photon polarization state to a single solid-state nuclear spin that has a coherence time of over 10 s. The storage process is achieved by coherently transferring the polarization state of a photon to an entangled electron–nuclear spin state of a nitrogen–vacancy centre in diamond. The nuclear spin-based optical quantum memory demonstrated here paves the way towards an absorption-based quantum repeater network.

  10. Functional Connectivity Estimated from Resting-State fMRI Reveals Selective Alterations in Male Adolescents with Pure Conduct Disorder

    PubMed Central

    Lu, Feng-Mei; Zhou, Jian-Song; Zhang, Jiang; Xiang, Yu-Tao; Zhang, Jian; Liu, Qi; Wang, Xiao-Ping; Yuan, Zhen

    2015-01-01

    Conduct disorder (CD) is characterized by a persistent pattern of antisocial behavior and aggression in childhood and adolescence. Previous task-based and resting-state functional magnetic resonance imaging (fMRI) studies have revealed widespread brain regional abnormalities in adolescents with CD. However, whether the resting-state networks (RSNs) are altered in adolescents with CD remains unknown. In this study, resting-state fMRI data were first acquired from eighteen male adolescents with pure CD and eighteen age- and gender-matched typically developing (TD) individuals. Independent component analysis (ICA) was implemented to extract nine representative RSNs, and the generated RSNs were then compared to show the differences between the CD and TD groups. Interestingly, it was observed from the brain mapping results that compared with the TD group, the CD group manifested decreased functional connectivity in four representative RSNs: the anterior default mode network (left middle frontal gyrus), which is considered to be correlated with impaired social cognition, the somatosensory network (bilateral supplementary motor area and right postcentral gyrus), the lateral visual network (left superior occipital gyrus), and the medial visual network (right fusiform, left lingual gyrus and right calcarine), which are expected to be relevant to the perceptual systems responsible for perceptual dysfunction in male adolescents with CD. Importantly, the novel findings suggested that male adolescents with pure CD were identified to have dysfunctions in both low-level perceptual networks (the somatosensory network and visual network) and a high-order cognitive network (the default mode network). Revealing the changes in the functional connectivity of these RSNs enhances our understanding of the neural mechanisms underlying the modulation of emotion and social cognition and the regulation of perception in adolescents with CD. PMID:26713867

  11. Laser-induced polarization of a quantum spin system in the steady-state regime

    NASA Astrophysics Data System (ADS)

    Zvyagin, A. A.

    2016-05-01

    The effect of the circularly polarized laser field on quantum spin systems in the steady-state regime, in which relaxation plays the central role, has been studied. The dynamical mean-field-like theory predicts several general results for the behavior of the time-average magnetization caused by the laser field. The induced magnetization oscillates with the frequency of the laser field (while Rabi-like oscillations, which modulate the latter in the dynamical regime, are damped by the relaxation in the steady-state regime). At high frequencies, that magnetization is determined by the value to which the relaxation process is directed. At low frequencies the slope of that magnetization as a function of the frequency is determined by the strength of the laser field. The anisotropy determines the resonance behavior of the time-averaged magnetization in both the ferromagnetic and antiferromagnetic cases with nonzero magnetic anisotropy. Nonlinear effects (in the magnitude of the laser field) have been considered. The effect of the laser field on quantum spin systems is maximal in resonance, where the time-averaged magnetization, caused by the laser field, is changed essentially. Out of resonance the changes in the magnetization are relatively small. The resonance effect is caused by the nonzero magnetic anisotropy. The resonance frequency is small (proportional to the anisotropy value) for spin systems with ferromagnetic interactions and enhanced by exchange interactions in the spin systems with antiferromagnetic couplings. We show that it is worthwhile to study the laser-field-induced magnetization of quantum spin systems caused by the high-frequency laser field in the steady-state regime in "easy-axis" antiferromagnetic spin systems (e.g., in Ising-like antiferromagnetic spin-chain materials). The effects of the Dzyaloshinskii-Moriya interaction and the spin-frustration couplings (in the case of the zigzag spin chain) have been analyzed.

  12. The Extended Crossover Peng-Robinson Equation of State for Describing the Thermodynamic Properties of Pure Fluids

    NASA Astrophysics Data System (ADS)

    Behnejad, Hassan; Cheshmpak, Hashem; Jamali, Asma

    2015-01-01

    In this paper, a theoretical method has been introduced for developing the crossover Peng-Robinson (CPR) equation of state (EoS) which incorporates the non-classical scaling laws asymptotically near the critical point into a classical analytic equation further away from the critical point. The CPR EoS has been adopted to describe the thermodynamic properties of some pure fluids (normal alkanes from methane to n-butane and carbon dioxide) such as density, saturated pressure, isochoric heat capacity and speed of sound. Unlike the original method for the crossover transformation made by Chen et al. (Phys Rev A 42:4470-4484, 1990), we have proposed a procedure which adding an additional term into the crossover transformation to obtain the thermophysical properties at the critical point more exactly. It is shown that this new crossover method yields a satisfactory representation of the thermodynamic properties close to the critical point for pure fluids relative to the original PR EoS.

  13. Density of states and Fisher's zeros in compact U(1) pure gauge theory

    NASA Astrophysics Data System (ADS)

    Bazavov, A.; Berg, B. A.; Du, Daping; Meurice, Y.

    2012-03-01

    We present high-accuracy calculations of the density of states using multicanonical methods for lattice gauge theory with a compact gauge group U(1) on 44, 64, and 84 lattices. We show that the results are consistent with weak and strong coupling expansions. We present methods based on Chebyshev interpolations and Cauchy theorem to find the (Fisher’s) zeros of the partition function in the complex β=1/g2 plane. The results are consistent with reweighting methods whenever the latter are accurate. We discuss the volume dependence of the imaginary part of the Fisher’s zeros, the width and depth of the plaquette distribution at the value of β where the two peaks have equal height. We discuss strategies to discriminate between first- and second-order transitions and explore them with data at larger volume but lower statistics. Higher statistics and even larger lattices are necessary to draw strong conclusions regarding the order of the transition.

  14. Pseudospin Vortex-Antivortex States with Interwoven Spin Texture in Double Layer Quantum Hall Systems

    NASA Astrophysics Data System (ADS)

    Roostaei, B.; Bourassa, J.; Fertig, H.; Mullen, K.; Cote, R.

    2006-03-01

    Enhanced nuclear spin relaxation rates have been observed in recent experiments[1] on double layer quantum Hall systems near total filling factor νT=1. The effect is analogous to what happens in single layer systems, where a possible explanation lies in the development of a Skyrme crystal with low energy spin wave modes as the system is doped away from integer filling. Double layer systems are thought to support bimeron excitations, analogous to skyrmions but with layer indices playing the role of spin states. We demonstrate,within the Hartree-Fock approximation, that for low interlayer tunneling and large separations the bimerons reorganize into a vortex-antivortex lattice with an interwoven real spin texture. These states are most stable at large layer separation, where the introduction of the spin degree of freedom can relax an interlayer charge imbalance at the cores of the merons. The presence of the real spin texture produces a true spontaneously broken symmetry whose Goldstone modes can explain the enhancement of the nuclear spin relaxation. [1]I.B. Spielman et al., Phys. Rev. Lett. 94, 076803 (2005).

  15. Evolution of the phonon density of states of LaCoO3 over the spin state transition

    SciTech Connect

    Golosova, N. O.; Kozlenko, D. P.; Kolesnikov, Alexander I; Kazimirov, V. Yu.; Smirnov, M. B.; Jirak, Z.; Savenko, B. N.

    2011-01-01

    The phonon spectra of LaCoO3 were studied by inelastic neutron scattering in the temperature range of 4 120 K. The DFT calculations of the lattice dynamics have been made for interpretation of the experimental data. The observed and calculated phonon frequencies were found to be in a reasonable agreement. The evolution of the phonon density of states over the spin state transition was analyzed. In the low-temperature range (T < 50 K), an increase in the energy of resolved breathing, stretching, and bending phonon modes was found, followed by their softening and broadening at higher temperatures due to the spin state transition and relevant orbital-phonon coupling.

  16. Electric field control of spin-resolved edge states in graphene quantum nanorings

    SciTech Connect

    Farghadan, R.; Saffarzadeh, A.

    2014-05-07

    The electric-field effect on the electronic and magnetic properties of triangular and hexagonal graphene quantum rings with zigzag edge termination is investigated by means of the single-band tight-binding Hamiltonian and the mean-field Hubbard model. It is shown how the electron and spin states in the nanoring structures can be manipulated by applying an electric field. We find different spin-depolarization behaviors with variation of electric field strength due to the dependence of spin densities on the shapes and edges of this kind of nanorings. In the case of triangular quantum rings, the magnetization on the inner and outer edges can be selectively tuned and the spin states depolarize gradually as the field strength is increased, while in the case of hexagonal nanorings, the transverse electric field reduces the magnetic moments on both inner and outer edges symmetrically and rapidly.

  17. Entangled collective-spin states of atomic ensembles under nonuniform atom-light interaction

    NASA Astrophysics Data System (ADS)

    Hu, Jiazhong; Chen, Wenlan; Vendeiro, Zachary; Zhang, Hao; Vuletić, Vladan

    2015-12-01

    We consider the optical generation and characterization of entanglement in atomic ensembles under nonuniform interaction between the ensemble and an optical mode. We show that for a wide range of parameters a system of nonuniformly coupled atomic spins can be described as an ensemble of uniformly coupled spins with a reduced effective atom-light coupling and a reduced effective atom number, with a reduction factor of order unity given by the ensemble-mode geometry. This description is valid even for complex entangled states with arbitrary phase-space distribution functions as long as the average total spin remains large, and the detection does not resolve single spins. Furthermore, we derive an analytic formula for determining the observable entanglement in the case, of relevance in practice, where the ensemble-mode coupling differs between state generation and measurement.

  18. In-beam spectroscopy of medium- and high-spin states in 133Ce

    NASA Astrophysics Data System (ADS)

    Ayangeakaa, A. D.; Garg, U.; Petrache, C. M.; Guo, S.; Zhao, P. W.; Matta, J. T.; Nayak, B. K.; Patel, D.; Janssens, R. V. F.; Carpenter, M. P.; Chiara, C. J.; Kondev, F. G.; Lauritsen, T.; Seweryniak, D.; Zhu, S.; Ghugre, S. S.; Palit, R.

    2016-05-01

    Medium and high-spin states in 133Ce were investigated using the 116Cd(22Ne, 5 n ) reaction and the Gammasphere array. The level scheme was extended up to an excitation energy of ˜22.8 MeV and spin 93/2 ℏ . Eleven bands of quadrupole transitions and two new dipole bands are identified. The connections to low-lying states of the previously known, high-spin triaxial bands were firmly established, thus fixing the excitation energy and, in many cases, the spin parity of the levels. Based on comparisons with cranked Nilsson-Strutinsky calculations and tilted axis cranking covariant density functional theory, it is shown that all observed bands are characterized by pronounced triaxiality. Competing multiquasiparticle configurations are found to contribute to a rich variety of collective phenomena in this nucleus.

  19. Spin-state transition induced half metallicity in a cobaltate from first principles

    NASA Astrophysics Data System (ADS)

    Ou, Xuedong; Fan, Fengren; Li, Zhengwei; Wang, Hongbo; Wu, Hua

    2016-02-01

    Half metal is a promising spintronic material. Here, we explore, using first principles calculations, a spin-state transition induced half metallicity in a layered cobaltate via a physical or chemical pressure. Our exemplary first principles study shows that the layered cobaltate Sr2CoO3F would undergo a transition, under a pressure of 5.4 GPa, from a high-spin antiferromagnetic insulator to an intermediate-spin ferromagnetic half-metal. The former phase is associated with a superexchange in a Mott insulator, and the latter one is due to a broad band formation and a kinetic energy gain of the partially occupied eg orbital. Note that the above transition could also be induced by a chemical pressure via doping in (Sr1-xCax)2CoO3F (x > 0.3). This work suggests that a cobaltate would be of a particular interest if stabilized into an intermediate-spin state.

  20. Towards a scalable quantum computation platform with solid-state spins in low temperature

    NASA Astrophysics Data System (ADS)

    Zhang, Wengang

    2016-05-01

    Nitrogen-vacancy (NV) center can be treated as an ``ion'' trapped in the diamond lattice. An electron spin triplet ground state (S = 1) of NV center can be polarized, coherently manipulated and detected. Together with hyperfine-coupled proximal Carbon-13 and Nitrogen-14 (15) nuclear spins, NV center acts as a promising platform for large scale quantum computation platform at room temperature. By cooling down the diamond to liquid-helium temperature (4K), phonons can be largely suppressed, giving us much longer spin relaxation time (T1) and coherence time (T2) compared with room temperature, and a possibility to readout electron spin state in a single shot. Here we report our progress in building up a prototype for a scalable diamond based quantum computer.

  1. Spin-transfer torque and specific features of magnetic-state switching in vacuum tunnel nanostructures

    SciTech Connect

    Demin, G. D. Popkov, A. F.; Dyuzhev, N. A.

    2015-12-15

    The specific features of spin-transfer torque in vacuum tunnel structures with magnetic electrodes are investigated using the quasi-classical Sommerfeld model of electron conductivity, which takes into account the exchange splitting of the spin energy subbands of free electrons. Using the calculated voltage dependences of the transferred torques for a tunnel structure with cobalt electrodes and noncollinear magnetic moments in the electrodes, diagrams of stable spin states on the current–field parameter plane in the in-plane geometry of the initial magnetization are obtained.

  2. Quantum state transfer between an optomechanical cavity and a diamond nuclear spin ensemble

    NASA Astrophysics Data System (ADS)

    Feng, Zhi-Bo; Wang, Hong-Ling; Yan, Run-Ying

    2016-08-01

    We explore an efficient scheme for transferring quantum state between an optomechanical cavity and nuclear spins of nitrogen-vacancy centers in diamond, where quantum information can be efficiently stored (retrieved) into (from) the nuclear spin ensemble assisted by a mechanical resonator in a dispersive regime. Our scheme works for a broad range of cavity frequencies and might have potential applications in employing the nuclear spin ensemble as a memory in quantum information processing. The feasibility of our protocol is analyzed using currently available parameters.

  3. LETTER TO THE EDITOR: Parity-broken ground state for the spin-1 pyrochlore antiferromagnet

    NASA Astrophysics Data System (ADS)

    Yamashita, Yasufumi; Ueda, Kazuo; Sigrist, Manfred

    2001-12-01

    The ground-state properties of the spin-1 pyrochlore antiferromagnet are studied by applying the VBS-like tetrahedron-unit decomposition to the original spin system. The symmetrization required on every vertex is taken into account by introducing a ferromagnetic coupling. The pairwise effective Hamiltonian between the adjacent tetrahedrons is obtained by considering the next nearest neighbour and the third neighbour exchange interactions. We find that the transverse component of the spin chirality exhibits a long-range order, breaking the parity symmetry of the tetrahedral group, while the chirality itself is not broken.

  4. Spin Equilibria in Monomeric Manganocenes: Solid State Magnetic and EXAFS Studies

    SciTech Connect

    Walter, M. D.; Sofield, C. D.; Booth, C. H.; Andersen, R. A.

    2009-02-09

    Magnetic susceptibility measurements and X-ray data confirm that tert-butyl-substituted manganocenes [(Me{sub 3}C){sub n}C{sub 5}H{sub 5?n}]{sub 2}Mn (n = 1, 2) follow the trend previously observed with the methylated manganocenes; that is, electron-donating groups attached to the Cp ring stabilize the low-spin (LS) electronic ground state relative to Cp{sub 2}Mn and exhibit higher spin-crossover (SCO) temperatures. However, introducing three CMe{sub 3} groups on each ring gives a temperature-invariant high-spin (HS) state manganocene. The origin of the high-spin state in [1,2,4-(Me{sub 3}C){sub 3}C{sub 5}H{sub 2}]{sub 2}Mn is due to the significant bulk of the [1,2,4-(Me{sub 3}C){sub 3}C{sub 5}H{sub 2}]{sup -} ligand, which is sufficient to generate severe inter-ring steric strain that prevents the realization of the low-spin state. Interestingly, the spin transition in [1,3-(Me{sub 3}C){sub 2}C{sub 5}H{sub 3}]{sub 2}Mn is accompanied by a phase transition resulting in a significant irreversible hysteresis ({Delta}T{sub c} = 16 K). This structural transition was also observed by extended X-ray absorption fine-structure (EXAFS) measurements. Magnetic susceptibility studies and X-ray diffraction data on SiMe{sub 3}-substituted manganocenes [(Me{sub 3}Si){sub n}C{sub 5}H{sub 5-n}]{sub 2}Mn (n = 1, 2, 3) show high-spin configurations in these cases. Although tetra- and hexasubstituted manganocenes are high-spin at all accessible temperatures, the disubstituted manganocenes exhibit a small low-spin admixture at low temperature. In this respect it behaves similarly to [(Me{sub 3}C)(Me{sub 3}Si)C{sub 5}H{sub 3}]{sub 2}Mn, which has a constant low-spin admixture up to 90 K and then gradually converts to high-spin. Thermal spin-trapping can be observed for [(Me{sub 3}C)(Me{sub 3}Si)C{sub 5}H{sub 3}]{sub 2}Mn on rapid cooling.

  5. Quantum state transfer between an optomechanical cavity and a diamond nuclear spin ensemble

    NASA Astrophysics Data System (ADS)

    Feng, Zhi-Bo; Wang, Hong-Ling; Yan, Run-Ying

    2016-05-01

    We explore an efficient scheme for transferring quantum state between an optomechanical cavity and nuclear spins of nitrogen-vacancy centers in diamond, where quantum information can be efficiently stored (retrieved) into (from) the nuclear spin ensemble assisted by a mechanical resonator in a dispersive regime. Our scheme works for a broad range of cavity frequencies and might have potential applications in employing the nuclear spin ensemble as a memory in quantum information processing. The feasibility of our protocol is analyzed using currently available parameters.

  6. Origin of Temperature Gradient in Nonequilibrium Steady States in Weakly Coupled Quantum Spin Systems

    NASA Astrophysics Data System (ADS)

    Ishida, Toyohiko; Sugita, Ayumu

    2016-07-01

    We study nonequilibrium steady states (NESSs) in quantum spin-1/2 chains in contact with two heat baths at different temperatures. We consider the weak-coupling limit both for spin-spin coupling in the system and for system-bath coupling. This setting allows us to treat NESSs with a nonzero temperature gradient analytically. We develop a perturbation theory for this weak-coupling situation and show a simple condition for the existence of nonzero temperature gradient. This condition is independent of the integrability of the system.

  7. Ground-state properties of linear-exchange quantum spin models

    NASA Astrophysics Data System (ADS)

    Danu, Bimla; Kumar, Brijesh; Pai, Ramesh V.

    2012-10-01

    We study a class of one-dimensional antiferromagnetic quantum spin-1/2 models using DMRG. The exchange interaction in these models decreases linearly with the separation between the spins, Jij = R - |i - j| for |i - j| < R, where R is a positive integer ⩾2. For |i - j| ⩾ R, the interaction is zero. It is known that all the odd-R models have the same exact dimer ground state as the Majumdar-Ghosh (MG) model. In fact, R = 3 is the MG model. However, for an even R, the exact ground state is not known in general, except for R = 2 (the integrable nearest-neighbor Heisenberg chain) and the asymptotic limit of R in which the MG dimer state emerges as the exact ground state. Therefore, we numerically study the ground-state properties of the finite even-R ≠ 2 models, particularly for R = 4, 6 and 8. We find that, unlike R = 2, the higher even-R models are spin-gapped, and exhibit robust dimer order of the MG type in the ground state. The spin-spin correlations decay rapidly to zero, albeit showing weak periodic revivals.

  8. Quantum antiferromagnetic Heisenberg half-odd-integer spin model as the entanglement Hamiltonian of the integer-spin Affleck-Kennedy-Lieb-Tasaki states

    NASA Astrophysics Data System (ADS)

    Rao, Wen-Jia; Zhang, Guang-Ming; Yang, Kun

    2016-03-01

    Applying a symmetric bulk bipartition to the one-dimensional Affleck-Kennedy-Lieb-Tasaki valence-bond solid (VBS) states for the integer spin-S Haldane gapped phase, we can create an array of fractionalized spin-S /2 edge states with the super unit cell l in the reduced bulk system, and the topological properties encoded in the VBS wave functions can be revealed. The entanglement Hamiltonian (EH) with even l corresponds to the quantum antiferromagnetic Heisenberg spin-S /2 model. For the even integer spins, the EH still describes the Haldane gapped phase. For the odd integer spins, however, the EH just corresponds to the quantum antiferromagnetic Heisenberg half-odd integer-spin model with spinon excitations, characterizing the critical point separating the topological Haldane phase from the trivial gapped phase. Our results thus demonstrate that the topological bulk property not only determines its fractionalized edge states but also the quantum criticality associated with the topological phase, where the elementary excitations are precisely those fractionalized edge degrees of freedom confined in the bulk of the topological phase.

  9. A simple modelling approach for prediction of standard state real gas entropy of pure materials.

    PubMed

    Bagheri, M; Borhani, T N G; Gandomi, A H; Manan, Z A

    2014-01-01

    The performance of an energy conversion system depends on exergy analysis and entropy generation minimisation. A new simple four-parameter equation is presented in this paper to predict the standard state absolute entropy of real gases (SSTD). The model development and validation were accomplished using the Linear Genetic Programming (LGP) method and a comprehensive dataset of 1727 widely used materials. The proposed model was compared with the results obtained using a three-layer feed forward neural network model (FFNN model). The root-mean-square error (RMSE) and the coefficient of determination (r(2)) of all data obtained for the LGP model were 52.24 J/(mol K) and 0.885, respectively. Several statistical assessments were used to evaluate the predictive power of the model. In addition, this study provides an appropriate understanding of the most important molecular variables for exergy analysis. Compared with the LGP based model, the application of FFNN improved the r(2) to 0.914. The developed model is useful in the design of materials to achieve a desired entropy value. PMID:25158071

  10. Formation of quantum spin Hall state on Si surface and energy gap scaling with strength of spin orbit coupling

    SciTech Connect

    Zhou, Miao; Ming, Wenmei; Liu, Zheng; Wang, Zhengfei; Yao, Yugui; Liu, Feng

    2014-11-19

    For potential applications in spintronics and quantum computing, it is desirable to place a quantum spin Hall insulator [i.e., a 2D topological insulator (TI)] on a substrate while maintaining a large energy gap. Here, we demonstrate a unique approach to create the large-gap 2D TI state on a semiconductor surface, based on first-principles calculations and effective Hamiltonian analysis. We show that when heavy elements with strong spin orbit coupling (SOC) such as Bi and Pb atoms are deposited on a patterned H-Si(111) surface into a hexagonal lattice, they exhibit a 2D TI state with a large energy gap of ≥0.5 eV. The TI state arises from an intriguing substrate orbital filtering effect that selects a suitable orbital composition around the Fermi level, so that the system can be matched onto a four-band effective model Hamiltonian. Furthermore, it is found that within this model, the SOC gap does not increase monotonically with the increasing strength of SOC. These interesting results may shed new light in future design and fabrication of large-gap topological quantum states.

  11. Formation of quantum spin Hall state on Si surface and energy gap scaling with strength of spin orbit coupling

    DOE PAGESBeta

    Zhou, Miao; Ming, Wenmei; Liu, Zheng; Wang, Zhengfei; Yao, Yugui; Liu, Feng

    2014-11-19

    For potential applications in spintronics and quantum computing, it is desirable to place a quantum spin Hall insulator [i.e., a 2D topological insulator (TI)] on a substrate while maintaining a large energy gap. Here, we demonstrate a unique approach to create the large-gap 2D TI state on a semiconductor surface, based on first-principles calculations and effective Hamiltonian analysis. We show that when heavy elements with strong spin orbit coupling (SOC) such as Bi and Pb atoms are deposited on a patterned H-Si(111) surface into a hexagonal lattice, they exhibit a 2D TI state with a large energy gap of ≥0.5more » eV. The TI state arises from an intriguing substrate orbital filtering effect that selects a suitable orbital composition around the Fermi level, so that the system can be matched onto a four-band effective model Hamiltonian. Furthermore, it is found that within this model, the SOC gap does not increase monotonically with the increasing strength of SOC. These interesting results may shed new light in future design and fabrication of large-gap topological quantum states.« less

  12. Formation of quantum spin Hall state on Si surface and energy gap scaling with strength of spin orbit coupling

    PubMed Central

    Zhou, Miao; Ming, Wenmei; Liu, Zheng; Wang, Zhengfei; Yao, Yugui; Liu, Feng

    2014-01-01

    For potential applications in spintronics and quantum computing, it is desirable to place a quantum spin Hall insulator [i.e., a 2D topological insulator (TI)] on a substrate while maintaining a large energy gap. Here, we demonstrate a unique approach to create the large-gap 2D TI state on a semiconductor surface, based on first-principles calculations and effective Hamiltonian analysis. We show that when heavy elements with strong spin orbit coupling (SOC) such as Bi and Pb atoms are deposited on a patterned H-Si(111) surface into a hexagonal lattice, they exhibit a 2D TI state with a large energy gap of ≥0.5 eV. The TI state arises from an intriguing substrate orbital filtering effect that selects a suitable orbital composition around the Fermi level, so that the system can be matched onto a four-band effective model Hamiltonian. Furthermore, it is found that within this model, the SOC gap does not increase monotonically with the increasing strength of SOC. These interesting results may shed new light in future design and fabrication of large-gap topological quantum states. PMID:25407432

  13. Conductimetric determination of phenylpropanolamine HCl, ranitidine HCl, hyoscyamine HBr and betaine HCl in their pure state and pharmaceutical preparations.

    PubMed

    Issa, Yousry M; Youssef, Ahmed F A; Mutair, Ali A

    2005-01-01

    Sodium tetraphenylborate and phosphotungstic acid were used as titrants for the conductimetric determination of phenylpropanolamine HCl (PPA.Cl), ranitidine HCl (Ra.Cl), hyoscyamine HBr (Hy.Br) and betaine HCl (Be.Cl) through ion-associate complex formation. The molar combining ratio and the solubility products of the formed ion-associates were studied and calculated. The suggested method has been applied to the determination of the mentioned drugs in their pure state and pharmaceutical preparations with mean recovery values of 97.71-102.97% and relative standard deviations 0.25-0.85%. The accuracy of the method is indicated by excellent recovery and low standard deviation. The results are compared with the pharmacopoeial or the official methods. PMID:15890349

  14. A computational study on choline benzoate and choline salicylate ionic liquids in the pure state and after CO2 adsorption.

    PubMed

    Aparicio, Santiago; Atilhan, Mert

    2012-08-01

    Choline-based ionic liquids show very adequate environmental, toxicological, and economical profiles for their application in many different technological areas. We report in this work a computational study on the properties of choline benzoate and choline salicylate ionic liquids, as representatives of this family of compounds, in the pure state and after CO(2) adsorption. Quantum chemistry calculations using the density functional theory approach for ionic pairs and ions, CO(2) pairs, were carried out, and the results analyzed using natural bond orbital and atoms in a molecule approaches. Classical molecular dynamics simulations of ionic liquids were done as a function of pressure, temperature, and CO(2) concentration. Microscopic structuring and intermolecular forces are analyzed together with the dynamic behavior of the studied fluids. PMID:22738425

  15. Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond

    SciTech Connect

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2015-08-24

    In this study, we demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ~0.7ms up to ~30ms. Furthermore, we extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We also identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.

  16. Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond

    DOE PAGESBeta

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2015-08-24

    In this study, we demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ~0.7ms up to ~30ms. Furthermore, we extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We also identify that the optimal controlmore » scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.« less

  17. Pseudospin vortex-antivortex states with interwoven spin textures in double-layer quantum Hall systems

    NASA Astrophysics Data System (ADS)

    Bourassa, J.; Roostaei, B.; Côté, R.; Fertig, H. A.; Mullen, K.

    2006-11-01

    Recent experiments on strongly correlated bilayer quantum Hall systems strongly suggest that, contrary to the usual assumption, the electron spin degree of freedom is not completely frozen either in the quantum Hall or in the compressibles states that occur at filling factor ν=1 . These experiments imply that the quasiparticles at ν=1 could have both spin and pseudospin textures; i.e., they could be CP3 Skyrmions. Using a microscopic unrestricted Hartree-Fock approximation, we compute the energy of several crystal states with spin, pseudospin, and mixed spin-pseudospin textures around ν=1 as a function of interlayer separation d for different values of tunneling (ΔSAS) , Zeeman (ΔZ) , and bias (Δb) energies. We show that in some range of these parameters, crystal states involving a certain amount of spin depolarization have lower energy than the fully spin-polarized crystals. We study this depolarization dependence on d , ΔSAS , ΔZ , and Δb and discuss how it can lead to the fast NMR relaxation rate observed experimentally.

  18. Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond

    NASA Astrophysics Data System (ADS)

    Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.

    2015-08-01

    We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ˜0.7 ms up to ˜30 ms . We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.

  19. Magnetic edge states and mixed-parity pairing in spin-triplet superconductors

    NASA Astrophysics Data System (ADS)

    Cuoco, Mario; Gentile, Paola; Noce, Canio; Vekhter, Ilya; Romano, Alfonso

    2014-03-01

    We show that a spontaneous magnetic moment may appear at the edge of a spin-triplet superconductor if the system allows for pairing in a subdominant channel and non-uniform spatial profile. To unveil the microscopic mechanism behind such effect we combine numerical solution of the Bogoliubov-De Gennes equations for a tight-binding model with nearest-neighbor attraction, and the symmetry based Ginzburg-Landau approach. We find that a modulation of the electronic density near the edge of the system leads to a non-unitary superconducting state where spin-singlet pairing coexists with the dominant triplet superconducting order. We demonstrate that the spin polarization at the edge appears due to the inhomogeneity of the non-unitary state and originates in the lifting of the spin-degeneracy of the Andreev bound-states. For chiral spin-triplet superconductors spin current flows along the interface and surface charge currents exhibit anomalous dependence on the magnetization. - A. Romano, P. Gentile, C. Noce, I. Vekhter, M. Cuoco, Phys. Rev. Lett. 110, 267002 (2013). This research has received funding from the EU -FP7/2007-2013 under grant agreement N. 264098 - MAMA, and was supported in part by US NSF via Grant No. DMR-1105339

  20. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet

    SciTech Connect

    Fu, Mingxuan; Imai, Takahashi; Han, Tian -Heng; Lee, Young S.

    2015-11-06

    Here, the kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χkagome, deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of χkagome that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.

  1. Ground-state information geometry and quantum criticality in an inhomogeneous spin model

    NASA Astrophysics Data System (ADS)

    Ma, Yu-Quan

    2015-09-01

    We investigate the ground-state Riemannian metric and the cyclic quantum distance of an inhomogeneous quantum spin-1/2 chain in a transverse field. This model can be diagonalized by using a general canonical transformation to the fermionic Hamiltonian mapped from the spin system. The ground-state Riemannian metric is derived exactly on a parameter manifold ring S1, which is introduced by performing a gauge transformation to the spin Hamiltonian through a twist operator. The cyclic ground-state quantum distance and the second derivative of the ground-state energy are studied in different exchange coupling parameter regions. Particularly, we show that, in the case of exchange coupling parameter Ja = Jb, the quantum ferromagnetic phase can be characterized by an invariant quantum distance and this distance will decay to zero rapidly in the paramagnetic phase. Project supported by the National Natural Science Foundation of China (Grant Nos. 11404023 and 11347131).

  2. Pure-state noninteracting v-representability of electron densities from Kohn-Sham calculations with finite basis sets

    NASA Astrophysics Data System (ADS)

    de Silva, Piotr; Wesolowski, Tomasz A.

    2012-03-01

    Within the linear combination of atomic orbitals (LCAO) approximation, one can distinguish two different Kohn-Sham potentials. One is the potential available numerically in calculations, and the other is the exact potential corresponding to the LCAO density. The latter is usually not available, but can be obtained from the total density by a numerical inversion procedure or, as is done here, analytically using only one LCAO Kohn-Sham orbital. In the complete basis-set limit, the lowest-lying Kohn-Sham orbital suffices to perform the analytical inversion, and the two potentials differ by no more than a constant. The relation between these two potentials is investigated here for diatomic molecules and several atomic basis sets of increasing size and quality. The differences between the two potentials are usually qualitative (wrong behavior at nuclear cusps and far from the molecule even if Slater-type orbitals are used) and δ-like features at nodal planes of the lowest-lying LCAO Kohn-Sham orbital. Such nodes occur frequently in LCAO calculations and are not physical. Whereas the behavior of the potential can be systematically improved locally by the increase of the basis sets, the occurrence of nodes is not correlated with the size of the basis set. The presence of nodes in the lowest-lying LCAO orbital can be used to monitor whether the effective potential in LCAO Kohn-Sham equations can be interpreted as the potential needed for pure-state noninteracting v-representability of the LCAO density. Squares of such node-containing lowest-lying LCAO Kohn-Sham orbitals are nontrivial examples of two-electron densities which are not pure-state noninteracting v-representable.

  3. Controllable Quantum State Transfer Between a Josephson Charge Qubit and an Electronic Spin Ensemble

    NASA Astrophysics Data System (ADS)

    Yan, Run-Ying; Wang, Hong-Ling; Feng, Zhi-Bo

    2016-01-01

    We propose a theoretical scheme to implement controllable quantum state transfer between a superconducting charge qubit and an electronic spin ensemble of nitrogen-vacancy centers. By an electro-mechanical resonator acting as a quantum data bus, an effective interaction between the charge qubit and the spin ensemble can be achieved in the dispersive regime, by which state transfers are switchable due to the adjustable electrical coupling. With the accessible experimental parameters, we further numerically analyze the feasibility and robustness. The present scheme could provide a potential approach for transferring quantum states controllably with the hybrid system.

  4. Diamond-nitrogen-vacancy electronic and nuclear spin-state anticrossings under weak transverse magnetic fields

    NASA Astrophysics Data System (ADS)

    Clevenson, Hannah; Chen, Edward H.; Dolde, Florian; Teale, Carson; Englund, Dirk; Braje, Danielle

    2016-08-01

    We report on detailed studies of electronic and nuclear spin states in the diamond-nitrogen-vacancy (NV) center under weak transverse magnetic fields. We numerically predict and experimentally verify a previously unobserved NV hyperfine level anticrossing (LAC) occurring at bias fields of tens of gauss—two orders of magnitude lower than previously reported LACs at ˜500 and ˜1000 G axial magnetic fields. We then discuss how the NV ground-state Hamiltonian can be manipulated in this regime to tailor the NV's sensitivity to environmental factors and to map into the nuclear spin state.

  5. Quantum entropy and uncertainty for two-mode squeezed, coherent and intelligent spin states

    NASA Technical Reports Server (NTRS)

    Aragone, C.; Mundarain, D.

    1993-01-01

    We compute the quantum entropy for monomode and two-mode systems set in squeezed states. Thereafter, the quantum entropy is also calculated for angular momentum algebra when the system is either in a coherent or in an intelligent spin state. These values are compared with the corresponding values of the respective uncertainties. In general, quantum entropies and uncertainties have the same minimum and maximum points. However, for coherent and intelligent spin states, it is found that some minima for the quantum entropy turn out to be uncertainty maxima. We feel that the quantum entropy we use provides the right answer, since it is given in an essentially unique way.

  6. Selective Equilibration of Spin-Polarized Quantum Hall Edge States in Graphene

    NASA Astrophysics Data System (ADS)

    Amet, F.; Williams, J. R.; Watanabe, K.; Taniguchi, T.; Goldhaber-Gordon, D.

    2014-05-01

    We report on transport measurements of dual-gated, single-layer graphene devices in the quantum Hall regime, allowing for independent control of the filling factors in adjoining regions. Progress in device quality allows us to study scattering between edge states when the fourfold degeneracy of the Landau level is lifted by electron correlations, causing edge states to be spin and/or valley polarized. In this new regime, we observe a dramatic departure from the equilibration seen in more disordered devices: edge states with opposite spins propagate without mixing. As a result, the degree of equilibration inferred from transport can reveal the spin polarization of the ground state at each filling factor. In particular, the first Landau level is shown to be spin polarized at half filling, providing an independent confirmation of a conclusion of Young et al. [Nat. Phys. 8, 550 (2012)]. The conductance in the bipolar regime is strongly suppressed, indicating that copropagating edge states, even with the same spin, do not equilibrate along PN interfaces. We attribute this behavior to the formation of an insulating ν =0 stripe at the PN interface.

  7. Quantum entanglement at ambient conditions in a macroscopic solid-state spin ensemble

    PubMed Central

    Klimov, Paul V.; Falk, Abram L.; Christle, David J.; Dobrovitski, Viatcheslav V.; Awschalom, David D.

    2015-01-01

    Entanglement is a key resource for quantum computers, quantum-communication networks, and high-precision sensors. Macroscopic spin ensembles have been historically important in the development of quantum algorithms for these prospective technologies and remain strong candidates for implementing them today. This strength derives from their long-lived quantum coherence, strong signal, and ability to couple collectively to external degrees of freedom. Nonetheless, preparing ensembles of genuinely entangled spin states has required high magnetic fields and cryogenic temperatures or photochemical reactions. We demonstrate that entanglement can be realized in solid-state spin ensembles at ambient conditions. We use hybrid registers comprising of electron-nuclear spin pairs that are localized at color-center defects in a commercial SiC wafer. We optically initialize 103 identical registers in a 40-μm3 volume (with 0.95−0.07+0.05 fidelity) and deterministically prepare them into the maximally entangled Bell states (with 0.88 ± 0.07 fidelity). To verify entanglement, we develop a register-specific quantum-state tomography protocol. The entanglement of a macroscopic solid-state spin ensemble at ambient conditions represents an important step toward practical quantum technology. PMID:26702444

  8. Quantum entanglement at ambient conditions in a macroscopic solid-state spin ensemble.

    PubMed

    Klimov, Paul V; Falk, Abram L; Christle, David J; Dobrovitski, Viatcheslav V; Awschalom, David D

    2015-11-01

    Entanglement is a key resource for quantum computers, quantum-communication networks, and high-precision sensors. Macroscopic spin ensembles have been historically important in the development of quantum algorithms for these prospective technologies and remain strong candidates for implementing them today. This strength derives from their long-lived quantum coherence, strong signal, and ability to couple collectively to external degrees of freedom. Nonetheless, preparing ensembles of genuinely entangled spin states has required high magnetic fields and cryogenic temperatures or photochemical reactions. We demonstrate that entanglement can be realized in solid-state spin ensembles at ambient conditions. We use hybrid registers comprising of electron-nuclear spin pairs that are localized at color-center defects in a commercial SiC wafer. We optically initialize 10(3) identical registers in a 40-μm(3) volume (with [Formula: see text] fidelity) and deterministically prepare them into the maximally entangled Bell states (with 0.88 ± 0.07 fidelity). To verify entanglement, we develop a register-specific quantum-state tomography protocol. The entanglement of a macroscopic solid-state spin ensemble at ambient conditions represents an important step toward practical quantum technology. PMID:26702444

  9. Dynamic control of spin states in interacting magnetic elements

    DOEpatents

    Jain, Shikha; Novosad, Valentyn

    2014-10-07

    A method for the control of the magnetic states of interacting magnetic elements comprising providing a magnetic structure with a plurality of interacting magnetic elements. The magnetic structure comprises a plurality of magnetic states based on the state of each interacting magnetic element. The desired magnetic state of the magnetic structure is determined. The active resonance frequency and amplitude curve of the desired magnetic state is determined. Each magnetic element of the magnetic structure is then subjected to an alternating magnetic field or electrical current having a frequency and amplitude below the active resonance frequency and amplitude curve of said desired magnetic state and above the active resonance frequency and amplitude curve of the current state of the magnetic structure until the magnetic state of the magnetic structure is at the desired magnetic state.

  10. Overlapping of heterogeneous and purely thermally activated solid-state processes in the combustion of a bituminous coal

    SciTech Connect

    Senneca, Osvalda; Salatino, Piero

    2006-02-01

    Mechanistic studies of coal combustion have long highlighted the variety of reaction pathways along which gasification may take place. These involve chemisorption of reactants, formation of surface oxides, surface mobility of chemisorbed species, and product desorption. At the same time, exposure of the solid fuel to high temperatures is associated with solid-state thermally activated processes. Altogether, the course of gasification may be profoundly affected by the overlapping and interplay of heterogeneous oxidation with purely thermally activated solid-state reactions. In the present work the combustion of a South African bituminous coal is analyzed in the framework of a simplified reaction network that embodies heterogeneous oxidative and thermally activated processes (pyrolysis, thermal annealing, coal combustion, char combustion, oxygen chemisorption) active both on the raw coal and on its char. The kinetics of each process of the network is assessed by a combination of thermogravimetric and gas analysis on coal and char samples. The analysis is directed to the determination of the prevailing combustion pathway, established from the interplay of oxidative and solid-state thermally activated processes, as a function of combustion conditions (temperature, heating rate, particle size). (author)

  11. Electronic transport in the quantum spin Hall state due to the presence of adatoms in graphene

    NASA Astrophysics Data System (ADS)

    Lima, Leandro; Lewenkopf, Caio

    Heavy adatoms, even at low concentrations, are predicted to turn a graphene sheet into a topological insulator with substantial gap. The adatoms mediate the spin-orbit coupling that is fundamental to the quantum spin Hall effect. The adatoms act as local spin-orbit scatterer inducing hopping processes between distant carbon atoms giving origin to transverse spin currents. Although there are effective models that describe spectral properties of such systems with great detail, quantitative theoretical work for the transport counterpart is still lacking. We developed a multiprobe recursive Green's function technique with spin resolution to analyze the transport properties for large geometries. We use an effective tight-binding Hamiltonian to describe the problem of adatoms randomly placed at the center of the honeycomb hexagons, which is the case for most transition metals. Our choice of current and voltage probes is favorable to experiments since it filters the contribution of only one spin orientation, leading to a quantized spin Hall conductance of e2 / h . We also discuss the electronic propagation in the system by imaging the local density of states and the electronic current densities. The authors acknowledge the Brazilian agencies CNPq, CAPES, FAPERJ and INCT de Nanoestruturas de Carbono for financial support.

  12. Control of vibrational states by spin-polarized transport in a carbon nanotube resonator

    NASA Astrophysics Data System (ADS)

    Stadler, P.; Belzig, W.; Rastelli, G.

    2015-02-01

    We study spin-dependent transport in a suspended carbon nanotube quantum dot in contact with two ferromagnetic leads and with the dot's spin coupled to the flexural mechanical modes. The spin-vibration interaction induces spin-flip processes between the two energy levels of the dot. This interaction arises from the spin-orbit coupling or a magnetic field gradient. The inelastic vibration-assisted spin flips give rise to a mechanical damping and, for an applied bias voltage, to a steady nonequilibrium occupation of the harmonic oscillator. We analyze these effects as function of the energy-level separation of the dot and the magnetic polarization of the leads. Depending on the magnetic configuration and the bias-voltage polarity, we can strongly cool a single mode or pump energy into it. In the latter case, we find that within our approximation, the system approaches eventually a regime of mechanical instability. Furthermore, owing to the sensitivity of the electron transport to the spin orientation, we find signatures of the nanomechanical motion in the current-voltage characteristic. Hence, the vibrational state can be read out in transport measurements.

  13. Electrical Spin Injection and Detection in Silicon: Effect of Interface States

    NASA Astrophysics Data System (ADS)

    Bearsdley, Jonas; Pu, Yong; Swartz, Adrian; Odenthal, Pat; Berger, Andrew; Ko, Dongkyun; Bhallamudi, Vidya; Hammel, Peter Christopher; Kawakami, Roland; Johnston-Halperin, Ezekiel; Pelz, Jon

    2012-02-01

    We have observed (using the local Hanle method) electrical spin injection into n and p type Si through a Fe/MgO/Si tunnel, with an effective spin lifetime of ˜130ps and an extremely large spin RA product as high as ˜0.1 Mφ*μm^2 at low bias and temperature. Both the spin-RA and the differential resistance decrease exponentially with bias at temperatures below 150K. The effective spin lifetime weakly depends on temperature, decreasing by ˜30% from 10K to 300K. We observe the inverse Hanle effect when an external magnetic field is applied parallel to the magnetization, possibly indicating the presence of stray fields near the Si surface. These observations roughly agree with other local Hanle spin injection studies in Silicon and GaAs, but differ strongly from the results expected for injection into bulk Silicon. The two stage tunneling model through localized states (LS) developed by Tran et al (PRL 102; p. 036601) can explain the large magnitude of the observed spin RA, and we have developed an extended LS model which can explain the voltage dependence, which will be discussed in another talk.

  14. Symmetry-selected spin-split hybrid states in C60/ferromagnetic interfaces

    NASA Astrophysics Data System (ADS)

    Li, Dongzhe; Barreteau, Cyrille; Kawahara, Seiji Leo; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Repain, Vincent; Smogunov, Alexander

    2016-02-01

    The understanding of orbital hybridization and spin polarization at the organic-ferromagnetic interface is essential in the search for efficient hybrid spintronic devices. Here, using first-principles calculations, we report a systematic study of spin-split hybrid states of C60 deposited on various ferromagnetic surfaces: bcc-Cr(001), bcc-Fe(001), bcc-Co(001), fcc-Co(001), and hcp-Co(0001). We show that the adsorption geometry of the molecule with respect to the surface crystallographic orientation of the magnetic substrate as well as the strength of the interaction play a crucial role in the spin polarization of the hybrid orbitals. We find that a large spin polarization in vacuum above the buckyball can only be achieved if the molecule is adsorbed upon a bcc-(001) surface by its pentagonal ring. Therefore, bcc-Cr(001), bcc-Fe(001), and bcc-Co(001) are the optimal candidates. Spin-polarized scanning tunneling spectroscopy measurements on single C60 adsorbed on Cr(001) and Co/Pt(111) also confirm that the symmetry both of the substrate and of the molecular conformation has a strong influence on the induced spin polarization. Our finding may give valuable insights for further engineering of spin filtering devices through single molecular orbitals.

  15. Three-spin interaction Ising model with a nondegenerate ground state at zero applied field

    NASA Astrophysics Data System (ADS)

    Bidaux, R.; Boccara, N.; Forgàcs, G.

    1986-10-01

    The field-temperature phase diagram of a two-dimensional, three-spin interaction Ising model is studied using two different methods: mean field approximation and numerical transfer matrix techniques. The former leads to a rather rich phase diagram in which two separate phases with different symmetries can be found, and which presents first-order transition lines, a triple point, and a critical end point, like the solid-liquid-gas phase diagram of a pure compound. The numerical transfer matrix study confirms part of these results, but does not clearly evidence the existence of the less symmetric phase.

  16. The ground state of a spin-1 anti-ferromagnetic atomic condensate for Heisenberg limited metrology

    NASA Astrophysics Data System (ADS)

    Wu, Ling-Na; You, Li

    2016-05-01

    The ground state of a spin-1 atomic condensate with anti-ferromagnetic interaction can be applied to quantum metrology approaching the Heisenberg limit. Unlike a ferromagnetic condensate state where individual atomic spins are aligned in the same direction, atoms in an anti-ferromagnetic ground state condensate exist as spin singlet pairs, whose inherent correlation promises metrological precisions beyond the standard quantum limit (SQL) for uncorrelated atoms. The degree of improvement over the SQL is measured by quantum Fisher information (QFI), whose dependence on the ratio of linear Zeeman shift p to spin-dependent atomic interaction c is studied. At a typical value of p = 0 . 4 c corresponding to a magnetic field of 28 . 6 μ G with c = h × 50 Hz (for 23 Na atom condensate in the F = 1 state at a typical density of ~1014cm-3), the scaled QFI can reach ~ 0 . 48 N , which is close to the limits of N for NooN state, or 0 . 5 N for twin-Fock state. We hope our work will stimulate experimental efforts towards reaching the anti-ferromagnetic condensate ground state at extremely low magnetic fields.

  17. Exact ground states of large two-dimensional planar Ising spin glasses

    NASA Astrophysics Data System (ADS)

    Pardella, G.; Liers, F.

    2008-11-01

    Studying spin-glass physics through analyzing their ground-state properties has a long history. Although there exist polynomial-time algorithms for the two-dimensional planar case, where the problem of finding ground states is transformed to a minimum-weight perfect matching problem, the reachable system sizes have been limited both by the needed CPU time and by memory requirements. In this work, we present an algorithm for the calculation of exact ground states for two-dimensional Ising spin glasses with free boundary conditions in at least one direction. The algorithmic foundations of the method date back to the work of Kasteleyn from the 1960s for computing the complete partition function of the Ising model. Using Kasteleyn cities, we calculate exact ground states for huge two-dimensional planar Ising spin-glass lattices (up to 30002 spins) within reasonable time. According to our knowledge, these are the largest sizes currently available. Kasteleyn cities were recently also used by Thomas and Middleton in the context of extended ground states on the torus. Moreover, they show that the method can also be used for computing ground states of planar graphs. Furthermore, we point out that the correctness of heuristically computed ground states can easily be verified. Finally, we evaluate the solution quality of heuristic variants of the L. Bieche approach.

  18. A state interaction spin-orbit coupling density matrix renormalization group method.

    PubMed

    Sayfutyarova, Elvira R; Chan, Garnet Kin-Lic

    2016-06-21

    We describe a state interaction spin-orbit (SISO) coupling method using density matrix renormalization group (DMRG) wavefunctions and the spin-orbit mean-field (SOMF) operator. We implement our DMRG-SISO scheme using a spin-adapted algorithm that computes transition density matrices between arbitrary matrix product states. To demonstrate the potential of the DMRG-SISO scheme we present accurate benchmark calculations for the zero-field splitting of the copper and gold atoms, comparing to earlier complete active space self-consistent-field and second-order complete active space perturbation theory results in the same basis. We also compute the effects of spin-orbit coupling on the spin-ladder of the iron-sulfur dimer complex [Fe2S2(SCH3)4](3-), determining the splitting of the lowest quartet and sextet states. We find that the magnitude of the zero-field splitting for the higher quartet and sextet states approaches a significant fraction of the Heisenberg exchange parameter. PMID:27334156

  19. A state interaction spin-orbit coupling density matrix renormalization group method

    NASA Astrophysics Data System (ADS)

    Sayfutyarova, Elvira R.; Chan, Garnet Kin-Lic

    2016-06-01

    We describe a state interaction spin-orbit (SISO) coupling method using density matrix renormalization group (DMRG) wavefunctions and the spin-orbit mean-field (SOMF) operator. We implement our DMRG-SISO scheme using a spin-adapted algorithm that computes transition density matrices between arbitrary matrix product states. To demonstrate the potential of the DMRG-SISO scheme we present accurate benchmark calculations for the zero-field splitting of the copper and gold atoms, comparing to earlier complete active space self-consistent-field and second-order complete active space perturbation theory results in the same basis. We also compute the effects of spin-orbit coupling on the spin-ladder of the iron-sulfur dimer complex [Fe2S2(SCH3)4]3-, determining the splitting of the lowest quartet and sextet states. We find that the magnitude of the zero-field splitting for the higher quartet and sextet states approaches a significant fraction of the Heisenberg exchange parameter.

  20. Meta-Atom Behavior in Clusters Revealing Large Spin Ground States.

    PubMed

    Hernández Sánchez, Raúl; Betley, Theodore A

    2015-11-01

    The field of single molecule magnetism remains predicated on super- and double exchange mechanisms to engender large spin ground states. An alternative approach to achieving high-spin architectures involves synthesizing weak-field clusters featuring close M-M interactions to produce a single valence orbital manifold. Population of this orbital manifold in accordance with Hund's rules could potentially yield thermally persistent high-spin ground states under which the valence electrons remain coupled. We now demonstrate this effect with a reduced hexanuclear iron cluster that achieves an S = 19/2 (χ(M)T ≈ 53 cm(3) K/mol) ground state that persists to 300 K, representing the largest spin ground state persistent to room temperature reported to date. The reduced cluster displays single molecule magnet behavior manifest in both variable-temperature zero-field (57)Fe Mössbauer and magnetometry with a spin reversal barrier of 42.5(8) cm(-1) and a magnetic blocking temperature of 2.9 K (0.059 K/min). PMID:26440452

  1. Non-collective high-spin states in /sup 148/Dy

    SciTech Connect

    Dines, E.L.

    1985-04-01

    General physical concepts regarding nuclear high-spin states are given. The high-spin states in /sup 148/Dy(Z = 66, N = 82) were produced via the reaction /sup 112/Cd(Pb-backed)(/sup 40/Ar,4n) at E/sub lab/ = 175, at the 88-inch Cyclotron at Lawrence Berkeley Laboratory. Methods for placing gates on various transitions above and below the 480 nsec isomer at 10/sup +/(known from previous work), as well as for calculating transition intensities and their associated errors, are given. Calculations of angular correlations for multiple ..gamma..-ray cascades, assuming non-zero-width distributions in m-states for some given spin state, were done and compared to experimental values. Analysis of RF - Ge and Ge - Ge TAC spectra for transitions above the 480 nsec isomer implied lifetimes of less than or equal to 5 nsec (except for the 327.2 keV transition). Using such analysis, some 19 new ..gamma..-ray transitions were discovered above the isomer, thereby extending the /sup 148/Dy level scheme up to spin I = 31 h-bar. Assignments of spins and parities for the new levels are made based on information obtained from angular correlations and the lifetime limits. Previous work on the 11 transitions below the 480 nsec isomer is confirmed.

  2. Separating the Spin States of a Free Electron Beam

    NASA Astrophysics Data System (ADS)

    Rifkin, Neil

    2008-10-01

    In 1922 Otto Stern and Walther Gerlach set out to test the spacial quantization of the electron by passing a beam of neutral silver atoms through a transverse magnetic field. The interaction of the two projections of the electron's magnetic moment with the magnetic field resulted in a splitting of the beam. However, for some sixty years it was generally accepted that the spin of free electrons, and thus their magnetic moment, could not be measured with an experiment similar to that of Stern and Gerlach. The reason being that the lorentz force on charged particles is far greater than the force due to the magnetic moment of the electron, thus blurring any desired results. To reduce the lorentz force, the electrons could be passed through a magnetic field whose gradient is in the direction of the electrons' momentum. This longitudinal Stern-Gerlach device, with a superconducting magnet, could polarize the tails of a low energy electron beam.

  3. Spin Superfluidity in the ν =0 Quantum Hall State of Graphene

    NASA Astrophysics Data System (ADS)

    Takei, So; Yacoby, Amir; Halperin, Bertrand I.; Tserkovnyak, Yaroslav

    2016-05-01

    Strong electron interactions can lead to a variety of broken-symmetry phases in monolayer graphene. In the quantum Hall regime, the interaction effect are enhanced by the formation of highly degenerate Landau levels, catalyzing the emergence of such phases. Recent magnetotransport studies show evidence that the ν =0 quantum Hall state of graphene is in an insulating canted antiferromagnetic phase with the Néel vector lying within the graphene plane. Here, we show that this Néel order can be detected via two-terminal spin transport. We find that a dynamic and inhomogeneous texture of the Néel vector can mediate nearly dissipationless (superfluid) transport of spin angular momentum polarized along the z axis, which could serve as a strong support for the antiferromagnetic scenario. The injection and detection of spin current in the ν =0 region can be achieved using the two spin-polarized edge channels of the |ν |=2 quantum Hall state. Measurements of the dependence of the spin current on the length of the ν =0 region would provide direct evidence for spin superfluidity.

  4. Chemistry and physics of the Earth's lower mantle influenced by iron spin and valence states

    NASA Astrophysics Data System (ADS)

    Xu, S.; Lin, J.; Morgan, D.

    2013-12-01

    Abstract: Earth's lower mantle is believed to be mainly made of (Al,Fe)-bearing silicate perovskite and ferropericlase in which the spin and valence states of iron can play a major role in our understanding of the physics and chemistry of the planet's interior. An ab-initio thermodynamic model has been used to predict the partitioning of iron in various spin and valence states, focusing on the effects of the spin transitions of Fe2+/Fe3+ and the Al3+ substitution in these major phases at relevant pressure-temperature and oxygen fugacity conditions. Our results show significant changes in the partition coefficient [KD=(Fe/Mg)Mg-Pv/(Fe/Mg)Fp] at the top lower-mantle conditions, and are further extended to understand the consequences of the dramatic changes in iron partitioning on lower mantle's density, bulk modulus and bulk sound speed. Our ab-initio simulations demonstrate that the Al content in the silicate perovskite plays a critical role on the Fe partitioning and stabilizes Fe3+ in perovskite through the coupled substitution of Fe3+-Al3+. The effects of the high-spin to low-spin transition of Fe2+ in ferropericlase and Fe3+ in perosvkite are explored. Based on a pyrolitic compositional model along an expected lower-mantle geotherm, we will present how the variations in iron spin and valences affect lower-mantle geophysics and geochemistry.

  5. Fractalization drives crystalline states in a frustrated spin system

    SciTech Connect

    Harrison, Neil; Sengupta, Pinaki; Batista, Cristian; Sebastian, Suchitra

    2008-01-01

    The fractalized Hofstadter butterfly energy spectrum predicted for magnetically confined fermions diffracted by a crystal lattice has remained beyond the reach of laboratory-accessible magnetic fields. We find the geometrically frustrated spin system SrCu{sub 2}(BO{sub 3}){sub 2} to provide a sterling demonstration of a system in which bosons confined by a magnetic and lattice potential mimic the behavior of fermions in the extreme quantum limit, giving rise to a sequence of plateaus at all magnetization m{sub z}/M{sub sat} = 1/q ratios 9 {>=} q {>=} 2 and p/q = 2/9 (m{sub sat} is the saturation magnetization) in magnetic fields up to 85 T and temperatures down to 29 mK, within the sequence of previously identified plateaus at 1/8, 1/4, and 1/3 of the saturated magnetization. We identify this hierarchy of plateaus as a consequence of confined bosons in SrCu{sub 2}(BO{sub 3}){sub 2} mimicking the high magnetic field fractalization predicted by the Hofstadter butterfly for fermionic systems. Such an experimental realization of the Hofstadter problem for interacting fermions has not been previously achieved in real materials, given the unachievably high magnetic flux densities or large lattice periods required. By a theoretical treatment that includes short-range repulsion in the Hofstadter treatment, stripe-like spin density-modulated phases are revealed in SrCu{sub 2}(BO{sub 3}){sub 2} as emergent from a fluidic fractal spectrum.

  6. Spin-helical Dirac states in graphene induced by polar-substrate surfaces with giant spin-orbit interaction: a new platform for spintronics

    PubMed Central

    Eremeev, S. V.; Nechaev, I. A.; Echenique, P. M.; Chulkov, E. V.

    2014-01-01

    Spintronics, or spin electronics, is aimed at efficient control and manipulation of spin degrees of freedom in electron systems. To comply with demands of nowaday spintronics, the studies of electron systems hosting giant spin-orbit-split electron states have become one of the most important problems providing us with a basis for desirable spintronics devices. In construction of such devices, it is also tempting to involve graphene, which has attracted great attention because of its unique and remarkable electronic properties and was recognized as a viable replacement for silicon in electronics. In this case, a challenging goal is to lift spin degeneracy of graphene Dirac states. Here, we propose a novel pathway to achieve this goal by means of coupling of graphene and polar-substrate surface states with giant Rashba-type spin-splitting. We theoretically demonstrate it by constructing the graphene@BiTeCl system, which appears to possess spin-helical graphene Dirac states caused by the strong interaction of Dirac and Rashba electrons. We anticipate that our findings will stimulate rapid growth in theoretical and experimental investigations of graphene Dirac states with real spin-momentum locking, which can revolutionize the graphene spintronics and become a reliable base for prospective spintronics applications. PMID:25365945

  7. Electric dipole transitions between Gamow-Teller and spin-dipole states

    SciTech Connect

    Suzuki, T.; Sagawa, H.; Van Giai, N.

    1998-01-01

    We study electric dipole transitions between Gamow-Teller (GT) and spin-dipole (SD) states. SD and GT excitations are calculated within the Hartree-Fock+Tamm-Dancoff approximation for {sup 48}Sc and {sup 90}Nb. The electric dipole transitions are found to be rather selective, and strong E1 transitions occur to some specific spin-dipole states. Calculated E1 transition strengths between GT and SD states are compared with the analytic sum rules within one-particle{endash}one-hole (1p-1h) configuration space and within both 1p-1h and 2p-2h model space. Possible implications for charge-exchange reactions may help to understand the quenching problem of spin excitations. {copyright} {ital 1998} {ital The American Physical Society}

  8. Suppression of spin-state transition in epitaxially strained LaCoO3

    NASA Astrophysics Data System (ADS)

    Pinta, C.; Fuchs, D.; Merz, M.; Wissinger, M.; Arac, E.; v. Löhneysen, H.; Samartsev, A.; Nagel, P.; Schuppler, S.

    2008-11-01

    Epitaxial thin films of LaCoO3 (e-LCO) exhibit ferromagnetic order with a transition temperature TC=85K while polycrystalline thin LaCoO3 films (p-LCO) remain paramagnetic. The temperature-dependent spin-state structure for both e-LCO and p-LCO was studied by x-ray absorption spectroscopy at the CoL2,3 and OK edges. Considerable spectral redistributions over temperature are observed for p-LCO . The spectra for e-LCO , on the other hand, do not show any significant changes for temperatures between 30 and 450 K at both edges, indicating that the spin state remains constant and that the epitaxial strain inhibits any population of the low-spin (S=0) state with decreasing temperature. This observation identifies an important prerequisite for ferromagnetism in e-LCO thin films.

  9. Surface-State Spin Textures and Mirror Chern Numbers in Topological Kondo Insulators

    NASA Astrophysics Data System (ADS)

    Legner, Markus; Rüegg, Andreas; Sigrist, Manfred

    2015-10-01

    The recent discovery of topological Kondo insulators has triggered renewed interest in the well-known Kondo insulator samarium hexaboride, which is hypothesized to belong to this family. In this Letter, we study the spin texture of the topologically protected surface states in such a topological Kondo insulator. In particular, we derive close relationships between (i) the form of the hybridization matrix at certain high-symmetry points, (ii) the mirror Chern numbers of the system, and (iii) the observable spin texture of the topological surface states. In this way, a robust classification of topological Kondo insulators and their surface-state spin texture is achieved. We underpin our findings with numerical calculations of several simplified and realistic models for systems like samarium hexaboride.

  10. Surface-State Spin Textures and Mirror Chern Numbers in Topological Kondo Insulators.

    PubMed

    Legner, Markus; Rüegg, Andreas; Sigrist, Manfred

    2015-10-01

    The recent discovery of topological Kondo insulators has triggered renewed interest in the well-known Kondo insulator samarium hexaboride, which is hypothesized to belong to this family. In this Letter, we study the spin texture of the topologically protected surface states in such a topological Kondo insulator. In particular, we derive close relationships between (i) the form of the hybridization matrix at certain high-symmetry points, (ii) the mirror Chern numbers of the system, and (iii) the observable spin texture of the topological surface states. In this way, a robust classification of topological Kondo insulators and their surface-state spin texture is achieved. We underpin our findings with numerical calculations of several simplified and realistic models for systems like samarium hexaboride. PMID:26550740

  11. Spin-State Tuning at Pseudo-tetrahedral d(6) Ions: Spin Crossover in [BP3]Fe(II)-X Complexes.

    PubMed

    Creutz, Sidney E; Peters, Jonas C

    2016-04-18

    Low-coordinate transition-metal complexes that undergo spin crossover remain rare. We report here a series of four-coordinate, pseudo-tetrahedral P3FeII–X complexes supported by tris(phosphine)borate P3 ([PhBP3R]−) and phosphiniminato X-type ligands (−N═PR3′) that, in combination, tune the spin-crossover behavior of the system. Most of the reported iron complexes undergo spin crossover at temperatures near or above room temperature in solution and in the solid state. The change in spin state coincides with a significant change in the degree of π-bonding between Fe and the bound N atom of the phosphiniminato ligand. Spin crossover is accompanied by striking changes in the ultraviolet–visible (UV-vis) absorption spectra, which allows for quantitative modeling of the thermodynamic parameters of the spin equilibria. These spin equilibria have also been studied by numerous techniques including paramagnetic nuclear magnetic resonance (NMR), infrared, and Mössbauer spectroscopies; X-ray crystallography; and solid-state superconducting quantum interference device (SQUID) magnetometry. These studies allow qualitative correlations to be made between the steric and electronic properties of the ligand substituents and the enthalpy and entropy changes associated with the spin equilibria. PMID:27042863

  12. Enantioselective Guest Effect on the Spin State of a Chiral Coordination Framework.

    PubMed

    Gural'skiy, Il'ya A; Kucheriv, Olesia I; Shylin, Sergii I; Ksenofontov, Vadim; Polunin, Ruslan A; Fritsky, Igor O

    2015-12-01

    The diversity of spin crossover (SCO) complexes that, on the one hand, display variable temperature, abruptness and hysteresis of the spin transition, and on the other hand, are spin-sensitive to the various guest molecules, makes these materials unique for the detection of different organic and inorganic compounds. We have developed a homochiral SCO coordination polymer with a spin transition sensitive to the inclusion of the guest 2-butanol, and these solvates with (R)- and (S)-alcohols demonstrate different SCO behaviours depending on the chirality of the organic analyte. A stereoselective response to the guest inclusion is detected as a shift in the temperature of the transition both from dia- to para- and from para- to diamagnetic states in heating and cooling modes respectively. Furthermore, the Mössbauer spectroscopy directly visualizes how the metallic centres in a chiral coordination framework differently sense the interaction with guests of different chiralities. PMID:26477972

  13. Steady-state hydrodynamics of a viscous incompressible fluid with spinning particles.

    PubMed

    Felderhof, B U

    2011-12-21

    The steady-state hydrodynamics of a viscous incompressible fluid with spinning particles is studied on the basis of extended Stokes equations. The profiles of flow velocity and spin velocity in simple flow situations may be used to determine the vortex viscosity and spin viscosity of the molecular liquid or fluid suspension. As an example, one situation studied is the flow generated by a uniform torque density in a planar layer of infinite fluid. The spinning particles drive a nearly uniform flow on either side of the layer, in opposite directions on the two sides. The Green function of the extended Stokes equations is derived. The translational and rotational friction coefficients of a sphere with no-slip boundary conditions, and the corresponding flow profiles, are calculated. PMID:22191899

  14. Engineered spin-state transitions of two interacting electrons in semiconductor nanowire quantum dots

    NASA Astrophysics Data System (ADS)

    Chen, Yan-Ting; Cheng, Shun-Jen; Tang, Chi-Shung

    2010-06-01

    Spin properties of two interacting electrons in a quantum dot (QD) embedded in a nanowire with controlled aspect ratio and longitudinal magnetic fields are investigated by using a configuration-interaction (CI) method. The developed CI theory based on a three-dimensional parabolic model provides explicit formulations of the Coulomb matrix elements and allows for straightforward and efficient numerical implementation. Our studies reveal fruitful features of spin-singlet-triplet transitions of two electrons confined in a nanowire QD, as a consequence of the competing effects of geometry-controlled kinetic-energy quantization, Coulomb interaction, and spin-Zeeman energy. The developed theory is further employed to study various spin states of two quantum-confined electrons in the regime of “crossover” dimensionality, from quasi-two-dimensional (disklike) QDs to finite one-dimensional (rodlike) QDs.

  15. On the truncation of the number of excited states in density functional theory sum-over-states calculations of indirect spin spin coupling constants

    SciTech Connect

    Zarycz, M. Natalia C. Provasi, Patricio F.; Sauer, Stephan P. A.

    2015-12-28

    It is investigated, whether the number of excited (pseudo)states can be truncated in the sum-over-states expression for indirect spin-spin coupling constants (SSCCs), which is used in the Contributions from Localized Orbitals within the Polarization Propagator Approach and Inner Projections of the Polarization Propagator (IPPP-CLOPPA) approach to analyzing SSCCs in terms of localized orbitals. As a test set we have studied the nine simple compounds, CH{sub 4}, NH{sub 3}, H{sub 2}O, SiH{sub 4}, PH{sub 3}, SH{sub 2}, C{sub 2}H{sub 2}, C{sub 2}H{sub 4}, and C{sub 2}H{sub 6}. The excited (pseudo)states were obtained from time-dependent density functional theory (TD-DFT) calculations with the B3LYP exchange-correlation functional and the specialized core-property basis set, aug-cc-pVTZ-J. We investigated both how the calculated coupling constants depend on the number of (pseudo)states included in the summation and whether the summation can be truncated in a systematic way at a smaller number of states and extrapolated to the total number of (pseudo)states for the given one-electron basis set. We find that this is possible and that for some of the couplings it is sufficient to include only about 30% of the excited (pseudo)states.

  16. On the truncation of the number of excited states in density functional theory sum-over-states calculations of indirect spin spin coupling constants

    NASA Astrophysics Data System (ADS)

    Zarycz, M. Natalia C.; Provasi, Patricio F.; Sauer, Stephan P. A.

    2015-12-01

    It is investigated, whether the number of excited (pseudo)states can be truncated in the sum-over-states expression for indirect spin-spin coupling constants (SSCCs), which is used in the Contributions from Localized Orbitals within the Polarization Propagator Approach and Inner Projections of the Polarization Propagator (IPPP-CLOPPA) approach to analyzing SSCCs in terms of localized orbitals. As a test set we have studied the nine simple compounds, CH4, NH3, H2O, SiH4, PH3, SH2, C2H2, C2H4, and C2H6. The excited (pseudo)states were obtained from time-dependent density functional theory (TD-DFT) calculations with the B3LYP exchange-correlation functional and the specialized core-property basis set, aug-cc-pVTZ-J. We investigated both how the calculated coupling constants depend on the number of (pseudo)states included in the summation and whether the summation can be truncated in a systematic way at a smaller number of states and extrapolated to the total number of (pseudo)states for the given one-electron basis set. We find that this is possible and that for some of the couplings it is sufficient to include only about 30% of the excited (pseudo)states.

  17. Two successive spin transitions in a wide range of pressure and coexistence of high- and low-spin states in clinoferrosilite FeSiO3

    NASA Astrophysics Data System (ADS)

    Dyachenko, Alexey A.; Shorikov, Alexey O.; Lukoyanov, Alexey V.; Anisimov, Vladimir I.

    2016-06-01

    We present a theoretical study of spectral and magnetic properties of clinoferrosilite FeSiO3. Within the DFT+DMFT method combining local density approximation with dynamical mean-field theory FeSiO3 was investigated in a wide range of pressure and temperature including the lower Earth's mantle conditions. For clinoferrosilite, which crystallizes in a monoclinic crystal structure, we predict two high-spin to low-spin transitions under pressure in the Fe-3 d shell with a crossover region at moderate temperatures, which becomes much broader at higher temperatures. An analysis of the Fe electronic configurations reveals that in clinoferrosilite the low- and high-spin states are predominantly involved and coexist in the spin crossover region, while a small amount of the intermediate spin states appears only at very high pressures and can be attributed to the distorted crystal structure of clinoferrosilite FeSiO3.

  18. Cooling into the spin-nematic state for a spin-1 Bose gas in an optical lattice

    SciTech Connect

    Chung, M.-C.; Yip Sungkit

    2009-05-15

    The possibility of adiabatically cooling a spin-1 polar Bose gas to a spin-nematic phase is theoretically discussed. The relation between the order parameter of the final spin-nematic phase and the starting temperature of the spinor Bose gas is obtained both using the mean-field approach for high temperature and spin-wave approach for low temperature. We find that there exists a good possibility to reach the spin-nematic ordering starting with spinor antiferromagnetic Bose gases.

  19. Spin dynamics in the modulation frame: application to homonuclear recoupling in magic angle spinning solid-state NMR.

    PubMed

    De Paëpe, Gaël; Lewandowski, Józef R; Griffin, Robert G

    2008-03-28

    We introduce a family of solid-state NMR pulse sequences that generalizes the concept of second averaging in the modulation frame and therefore provides a new approach to perform magic angle spinning dipolar recoupling experiments. Here, we focus on two particular recoupling mechanisms-cosine modulated rotary resonance (CMpRR) and cosine modulated recoupling with isotropic chemical shift reintroduction (COMICS). The first technique, CMpRR, is based on a cosine modulation of the rf phase and yields broadband double-quantum (DQ) (13)C recoupling using >70 kHz omega(1,C)/2pi rf field for the spinning frequency omega(r)/2=10-30 kHz and (1)H Larmor frequency omega(0,H)/2pi up to 900 MHz. Importantly, for p>or=5, CMpRR recouples efficiently in the absence of (1)H decoupling. Extension to lower p values (3.5spinning frequencies is possible using low power (1)H irradiation (<0.25 omega(r)/2pi). This phenomenon is explained through higher order cross terms including a homonuclear third spin assisted recoupling mechanism among protons. CMpRR mitigates the heating effects of simultaneous high power (13)C recoupling and (1)H decoupling. The second technique, COMICS, involves low power (13)C irradiation that induces simultaneous recoupling of the (13)C DQ dipolar and isotropic chemical shift terms. In contrast to CMpRR, where the DQ bandwidth (approximately 30 kHz at omega(0,H)/2pi=750 MHz) covers the entire (13)C spectral width, COMICS recoupling, through the reintroduction of the isotropic chemical shift, is selective with respect to the carrier frequency, having a typical bandwidth of approximately 100 Hz. This approach is intended as a general frequency selective method circumventing dipolar truncation (supplementary to R(2) experiments). These new gamma-encoded sequences with attenuated rf requirements extend the applicability of homonuclear recoupling techniques to new regimes--high spinning and Larmor frequencies--and therefore should be of major

  20. Pure phase decoherence in a ring geometry

    SciTech Connect

    Zhu, Z.; Aharony, A.; Entin-Wohlman, O.; Stamp, P. C. E.

    2010-06-15

    We study the dynamics of pure phase decoherence for a particle hopping around an N-site ring, coupled both to a spin bath and to an Aharonov-Bohm flux which threads the ring. Analytic results are found for the dynamics of the influence functional and of the reduced density matrix of the particle, both for initial single wave-packet states, and for states split initially into two separate wave packets moving at different velocities. We also give results for the dynamics of the current as a function of time.

  1. Quantum Bocce: Magnon-magnon collisions between propagating and bound states in 1D spin chains

    NASA Astrophysics Data System (ADS)

    Longo, Paolo; Greentree, Andrew D.; Busch, Kurt; Cole, Jared H.

    2013-08-01

    The dynamics of two magnons in a Heisenberg spin chain under the influence of a non-uniform magnetic field is investigated by means of a numerical wave-function-based approach using a Holstein-Primakoff transformation. The magnetic field is localized in space such that it supports exactly one single-particle bound state. We study the interaction of this bound mode with an incoming spin wave and the interplay between transmittance, energy and momentum matching. We find analytic criteria for maximizing the interconversion between propagating single-magnon modes and true propagating two-magnon states. The manipulation of bound and propagating magnons is an essential step towards quantum magnonics.

  2. Shape evolution at high spin states in Kr and Br isotopes

    SciTech Connect

    Trivedi, T.; Palit, R.; Naik, Z.; Jain, H. C.; Negi, D.; Kumar, R.; Singh, R. P.; Muralithar, S.; Pancholi, S. C.; Bhowmik, R. K.; Yang, Y.-C.; Sun, Y.; Sheikh, J. A.; Raja, M. K.; Kumar, S.; Choudhury, D.; Jain, A. K.; Mehrotra, I.

    2014-08-14

    The high spin states in A = 75, Kr and Br isotopes have been populated via fusion-evaporation reaction at an incident beam energy of 90 MeV. The de-exciting γ-rays were detected utilizing the Indian National Gamma Array (INGA). Lifetime of these excited high spin states were determined by Doppler-shift attenuation method. Experimental results obtained from lifetime measurement are interpreted in the frame work of projected shell-model to get better insight into the evolution of collectivity. Comparison of the calculations of the model with transitional quadrupole moments Q{sub t} of the positive and negative parity bands firmly established their configurations.

  3. Ground states of spin-2 condensates in an external magnetic field

    SciTech Connect

    Zheng, G.-P.; Tong, Y.-G.; Wang, F.-L.

    2010-06-15

    The possible ground states of spin-2 Bose-Einstein condensates in an external magnetic field are obtained analytically and classified systematically according to the population of the condensed atoms at the hyperfine sublevels. It is shown that the atoms can populate simultaneously at four hyperfine sublevels in a weak magnetic field with only the linear Zeeman energy, in contrast to that in a stronger magnetic field with the quadratic Zeeman energy, where condensed atoms can at most populate at three hyperfine sublevels in the ground states. Any spin configuration we obtained will give a closed subspace in the order parameter space of the condensates.

  4. Dimerized ground state in the one-dimensional spin-1 boson Hubbard model

    SciTech Connect

    Apaja, Vesa; Syljuaasen, Olav F.

    2006-09-15

    We have investigated the one-dimensional spin-1 boson Hubbard model with antiferromagnetic interactions using quantum Monte Carlo methods. We obtain the shapes of the two lowest Mott lobes and show that the ground state within the lowest Mott lobe is dimerized. The results presented here are relevant for optically trapped antiferromagnetic spin-1 bosons. An experimental signature of the dimerized ground state is modulated Bragg peaks in the noise distribution of the atomic cloud obtained after switching off the trap. These Bragg peaks are located at wave vectors corresponding to half-integer multiples of the reciprocal wave vector of the optical lattice.

  5. Nanoscale Mach-Zehnder interferometer with spin-resolved quantum Hall edge states

    NASA Astrophysics Data System (ADS)

    Karmakar, Biswajit; Venturelli, Davide; Chirolli, Luca; Giovannetti, Vittorio; Fazio, Rosario; Roddaro, Stefano; Pfeiffer, Loren N.; West, Ken W.; Taddei, Fabio; Pellegrini, Vittorio

    2015-11-01

    We realize a nanoscale-area Mach-Zehnder interferometer with co-propagating quantum Hall spin-resolved edge states and demonstrate the persistence of gate-controlled quantum interference oscillations, as a function of an applied magnetic field, at relatively large temperatures. Arrays of top-gate magnetic nanofingers are used to induce a resonant charge transfer between the pair of spin-resolved edge states. To account for the pattern of oscillations measured as a function of magnetic field and gate voltage, we have developed a simple theoretical model which satisfactorily reproduces the data.

  6. Influence of octupole interactions on the behavior of negative-parity states at low spins

    SciTech Connect

    Sitdikov, A. S. Safarov, R. Kh.; Kvasil, J.

    2006-12-15

    The energies of negative-parity levels based on two-particle states exhibit a nonlinear behavior at low spins versus the core-rotation energy because the alignment process has not yet been completed for them. This behavior of negative-parity levels in the low-spin region is satisfactorily described upon the inclusion of octupole-octupole interactions. This is demonstrated within the rotational model involving the Coriolis mixing of states for the even-even isotopes {sup 162-168}Hf.

  7. Electronic Spin and Valence States of Iron in the Lower-Mantle Silicate Perovskite

    NASA Astrophysics Data System (ADS)

    Chang, Y. Y.; Wu, Y.; Lin, J. F.; McCammon, C. A.; Okuchi, T.; Tomioka, N.

    2014-12-01

    Magnesium silicate perovskite (Pv) is the most abundant phase in the Earth's lower mantle and can make up to 75% in volume of the lower mantle in a pyrolitic compositional model. The electronic spin and valence states of iron (Fe) in Pv directly influence its physical and chemical properties, and therefore it is important to study the electronic spin and valence states of Fe in Pv at conditions corresponding to the Earth's lower mantle. Numerous studies have been dedicated to understanding the electronic spin and valence states of Fe in Pv at high pressures using experimental and theoretical techniques. However, experimental results and possible interpretations remain highly debated due to the multiple valence states and site occupancies of Fe in Pv. Previous studies also showed the incorporation of aluminum (Al) into a Fe-bearing Pv can affect the placement of Fe3+ and further complicate interpretations of experimental results. Here we present the experimental result on electronic spin and valence states of Fe using well-characterized single-crystal Fe-bearing and Al-Fe-bearing Pv to the pressures relevant to the lower mantle by synchrotron X-ray emission spectroscopy (XES) and Mössbauer spectroscopy (SMS). The samples used in this experiment were first characterized by Mössbauer spectroscopy (MS) at ambient conditions to identify the initial Fe electronic spin and valence states before performing high-pressure experiments. The XES spectra were analyzed using a new analytical method, integrate relative difference (IRD) method. The new IRD method had been shown in the previous study to be a more effective method of probing the pressure range of Fe spin transition and can avoid the influence of peak broadening on the interpretation of the spin states of Fe at high pressures. Our study will assist the comprehension and interpretation of the electronic spin and valence states of Fe on the major lower-mantle mineral. The result has implications to deep Earth

  8. Spin-orbit splitting of the Shockley surface state on Cu(111)

    NASA Astrophysics Data System (ADS)

    Tamai, A.; Meevasana, W.; King, P. D. C.; Nicholson, C. W.; de la Torre, A.; Rozbicki, E.; Baumberger, F.

    2013-02-01

    We present angle-resolved photoemission data from Cu(111). Using a focused 6 eV continuous-wave laser for photoexcitation, we achieve a high effective momentum resolution, enabling detection of the Rashba spin splitting in the Shockley surface state on Cu(111). The magnitude of the spin splitting of Δk˜0.006 Å-1 is surprisingly large and exceeds values predicted for the analogous surface state on Ag(111), but is reproduced by first-principles calculations. We further resolve a kink in the dispersion, which we attribute to electron-phonon coupling.

  9. Phase boundary of spin-polarized-current state of electrons in bilayer graphene

    NASA Astrophysics Data System (ADS)

    Yan, Xin-Zhong; Ma, Yinfeng; Ting, C. S.

    2016-06-01

    Using a four-band Hamiltonian, we study the phase boundary of spin-polarized-current state (SPCS) of interacting electrons in bilayer graphene. The model of spin-polarized-current state has previously been shown to resolve a number of experimental puzzles in bilayer graphene. The phase boundaries of the SPCS with and without the external voltage between the two layers are obtained in this work. An unusual phase boundary where there are two transition temperatures for a given carrier concentration is found at finite external voltage. The physics of this phenomenon is explained.

  10. Controlling the Excited-State Dynamics of Nuclear Spin Isomers Using the Dynamic Stark Effect.

    PubMed

    Waldl, Maria; Oppel, Markus; González, Leticia

    2016-07-14

    Stark control of chemical reactions uses intense laser pulses to distort the potential energy surfaces of a molecule, thus opening new chemical pathways. We use the concept of Stark shifts to convert a local minimum into a local maximum of the potential energy surface, triggering constructive and destructive wave-packet interferences, which then induce different dynamics on nuclear spin isomers in the electronically excited state of a quinodimethane derivative. Model quantum-dynamical simulations on reduced dimensionality using optimized ultrashort laser pulses demonstrate a difference of the excited-state dynamics of two sets of nuclear spin isomers, which ultimately can be used to discriminate between these isomers. PMID:26840424

  11. Dispersive measurement of electron spin states in Coulomb-confined silicon double quantum dots

    NASA Astrophysics Data System (ADS)

    House, Matthew; Kobayashi, Takashi; Weber, Bent; Hile, Sam; Rogge, Sven; Simmons, Michelle

    2015-03-01

    We use radio frequency reflectometry with a resonant circuit to investigate a double quantum dot device patterned by the placement of phosphorus donors in silicon with scanning tunnelling microscope lithography. The circuit responds to electron tunnelling to and from the quantum dots, the complex admittance of which provides information about the tunnel coupling between the dots and the leads. With four electrons on two dots, the Pauli Exclusion Principle makes tunnelling of one electron between the two dots spin dependent, which we exploit to measure the electronic spin state. We map the ground state transition between singlet and triplet states as a function of electric and magnetic fields, which shows that the exchange energy can be tuned over an order of magnitude (about 10 to 100 μeV) or more in this device. We apply high frequency pulses to induce an excited spin state and observe that the dispersive measurement can detect the excited spin state in addition to the ground state.

  12. Using the ground state of an antiferromagnetic spin-1 atomic condensate for Heisenberg-limited metrology

    NASA Astrophysics Data System (ADS)

    Wu, Ling-Na; You, L.

    2016-03-01

    We show that the ground state of a spin-1 atomic condensate with antiferromagnetic interactions constitutes a useful resource for quantum metrology upon approaching the Heisenberg limit. Unlike a ferromagnetic condensate state where individual atomic spins are aligned in the same direction, the antiferromagnetic ground-state condensate is a condensate of spin-singlet atom pairs. The inherent correlation between paired atoms allows for parameter estimation at precisions beyond the standard quantum limit (SQL) for uncorrelated atoms. The degree of improvement over the SQL is measured by the scaled quantum Fisher information (QFI), whose dependence on the ratio of linear Zeeman shift p to spin-dependent atomic interaction c is studied. At a typical value of p =0.4 c , which corresponds to a magnetic field of 28.6 μ G for c =50 h Hz (for 23Na atom condensate in the F =1 state at a typical density of ˜1014cm-3 ), the scaled QFI can reach ˜0.48 N , which approaches the limit of 0.5 N for the twin-Fock state |N/2 > +|N/2 > - . Our work encourages experimental efforts to reach the ground state of an antiferromagnetic condensate at a extremely low magnetic field.

  13. The Quantum Mixed-Spin Heme State of Barley Peroxidase: A Paradigm for Class III Peroxidases

    SciTech Connect

    Howes, B.D.; Ma, J.; Marzocchi, M.P.; Schiodt, C.B.; Shelnutt, J.A.; Smulevich, G.; Welinder, K.G.; Zhang, J.

    1999-03-23

    Electronic absorption and resonance Raman (RR) spectra of the ferric form of barley grain peroxidase (BP 1) at various pH values both at room temperature and 20 K are . reported, together with EPR spectra at 10 K. The ferrous forms and the ferric complex with fluoride have also been studied. A quantum mechanically mixed-spin (QS) state has been identified. The QS heme species co-exists with 6- and 5-cHS heroes; the relative populations of these three spin states are found to be dependent on pH and temperature. However, the QS species remains in all cases the dominant heme spin species. Barley peroxidase appears to be further characterized by a splitting of the two vinyl stretching modes, indicating that the vinyl groups are differently conjugated with the porphyrin. An analysis of the presently available spectroscopic data for proteins from all three peroxidase classes suggests that the simultaneous occurrence of the QS heme state as well as the splitting of the two vinyl stretching modes is confined to class III enzymes. The former point is discussed in terms of the possible influences of heme deformations on heme spin state. It is found that moderate saddling alone is probably not enough to cause the QS state, although some saddling maybe necessary for the QS state.

  14. Far-from-Equilibrium Field Theory of Many-Body Quantum Spin Systems: Prethermalization and Relaxation of Spin Spiral States in Three Dimensions

    NASA Astrophysics Data System (ADS)

    Babadi, Mehrtash; Demler, Eugene; Knap, Michael

    2015-10-01

    We study theoretically the far-from-equilibrium relaxation dynamics of spin spiral states in the three-dimensional isotropic Heisenberg model. The investigated problem serves as an archetype for understanding quantum dynamics of isolated many-body systems in the vicinity of a spontaneously broken continuous symmetry. We present a field-theoretical formalism that systematically improves on the mean field for describing the real-time quantum dynamics of generic spin-1 /2 systems. This is achieved by mapping spins to Majorana fermions followed by a 1 /N expansion of the resulting two-particle-irreducible effective action. Our analysis reveals rich fluctuation-induced relaxation dynamics in the unitary evolution of spin spiral states. In particular, we find the sudden appearance of long-lived prethermalized plateaus with diverging lifetimes as the spiral winding is tuned toward the thermodynamically stable ferro- or antiferromagnetic phases. The emerging prethermalized states are characterized by different bosonic modes being thermally populated at different effective temperatures and by a hierarchical relaxation process reminiscent of glassy systems. Spin-spin correlators found by solving the nonequilibrium Bethe-Salpeter equation provide further insight into the dynamic formation of correlations, the fate of unstable collective modes, and the emergence of fluctuation-dissipation relations. Our predictions can be verified experimentally using recent realizations of spin spiral states with ultracold atoms in a quantum gas microscope [S. Hild et al., Phys. Rev. Lett. 113, 147205 (2014), 10.1103/PhysRevLett.113.147205].

  15. Emergence of quantum spin Hall and ``half-topological'' states at Graphene/TMDC heterostructures

    NASA Astrophysics Data System (ADS)

    Kochan, Denis; Gmitra, Martin; Högl, Petra; Fabian, Jaroslav

    We discuss orbital and spin-orbital proximity effects emerging in graphene deposited on a monolayer transition-metal dichalcogenides (TMDCs: MoS2, MoSe2, WS2, WSe2) and analyze the impact on spin transport in such graphene/TMDC heterostructures. First-principles investigations show that graphene on MoS2, MoSe2, and WS2 has a topologically trivial band structure, while graphene on WSe2 exhibits inverted bands. The essential low energy physics can be well described by a symmetry inspired realistic tight-binding Hamiltonian. We predict topologically protected helical edge states for graphene zigzag nanoribbons on WSe2, demonstrating the emergence of the quantum spin Hall effect. Our model also features ''half-topological states'', which are protected against time-reversal disorder on one edge only. Unlike in pristine graphene, the proximity spin-orbit coupling in graphene on TMDCs is significant (orders of meV), making the predicted effect testable experimentally. References: M. Gmitra, D. Kochan, P. Högl, J. Fabian; Trivial and inverted Dirac bands, and emergence of quantum spin Hall states in graphene on transition-metal dichalcogenides, arXiv:1510.00166 This research was supported by DFG SFB 689, GRK 1570 and by the EU Seventh Framework Programme under Grant Agreement No. 604391 Graphene Flagship.

  16. Stability of a spin-triplet nematic state near to a quantum critical point

    NASA Astrophysics Data System (ADS)

    Hannappel, G.; Pedder, C. J.; Krüger, F.; Green, A. G.

    2016-06-01

    We analyze a model of itinerant electrons interacting through a quadrupole density-density repulsion in three dimensions. At the mean-field level, the interaction drives a continuous Pomeranchuk instability towards d -wave, spin-triplet nematic order, which simultaneously breaks the SU(2) spin-rotation and spatial-rotation symmetries. This order is characterized by spin-antisymmetric, elliptical deformations of the Fermi surfaces of up and down spins. We show that the effects of quantum fluctuations are similar to those in metallic ferromagnets, rendering the nematic transition first order at low temperatures. Using the fermionic quantum order-by-disorder approach to self-consistently calculate fluctuations around possible modulated states, we show that the first-order transition is preempted by the formation of a helical spin-triplet d -density wave. Such a state is closely related to d -wave bond density wave order in square-lattice systems. Moreover, we show that it may coexist with a modulated, p -wave superconducting state.

  17. Interpreting current-induced spin polarization in topological insulator surface states

    NASA Astrophysics Data System (ADS)

    Li, Pengke; Appelbaum, Ian

    2016-06-01

    Several recent experiments on three-dimensional topological insulators claim to observe a large charge current-induced nonequilibrium ensemble spin polarization of electrons in the helical surface state. We present a comprehensive criticism of such claims, using both theory and experiment: First, we clarify the interpretation of quantities extracted from these measurements by deriving standard expressions from a Boltzmann transport equation approach in the relaxation-time approximation at zero and finite temperature to emphasize our assertion that, despite high in-plane spin projection, obtainable current-induced ensemble spin polarization is minuscule. Second, we use a simple experiment to demonstrate that magnetic field-dependent open-circuit voltage hysteresis (identical to those attributed to current-induced spin polarization in topological insulator surface states) can be generated in analogous devices where current is driven through thin films of a topologically trivial metal. This result ipso facto discredits the naive interpretation of previous experiments with TIs, which were used to claim observation of helicity, i.e., spin-momentum locking in the topologically protected surface state.

  18. All possible coupling schemes in XY spin chains for perfect state transfer

    SciTech Connect

    Wang Yaoxiong; Shuang Feng; Rabitz, Herschel

    2011-07-15

    We investigate quantum state transfer in XY spin chains and propose a recursive procedure to construct the nonuniform couplings within these chains of arbitrary length in order to achieve perfect state transfer. We show that this method is capable of finding all possible coupling schemes for perfect state transfer. These schemes, without external control fields, involve analytically identified engineered couplings without the need for dynamical control. The analytical solutions provide all information for coupling design.

  19. Emergence of nontrivial magnetic excitations in a spin-liquid state of kagomé volborthite.

    PubMed

    Watanabe, Daiki; Sugii, Kaori; Shimozawa, Masaaki; Suzuki, Yoshitaka; Yajima, Takeshi; Ishikawa, Hajime; Hiroi, Zenji; Shibauchi, Takasada; Matsuda, Yuji; Yamashita, Minoru

    2016-08-01

    When quantum fluctuations destroy underlying long-range ordered states, novel quantum states emerge. Spin-liquid (SL) states of frustrated quantum antiferromagnets, in which highly correlated spins fluctuate down to very low temperatures, are prominent examples of such quantum states. SL states often exhibit exotic physical properties, but the precise nature of the elementary excitations behind such phenomena remains entirely elusive. Here, we use thermal Hall measurements that can capture the unexplored property of the elementary excitations in SL states, and report the observation of anomalous excitations that may unveil the unique features of the SL state. Our principal finding is a negative thermal Hall conductivity [Formula: see text] which the charge-neutral spin excitations in a gapless SL state of the 2D kagomé insulator volborthite Cu3V2O7(OH)2[Formula: see text]2H2O exhibit, in much the same way in which charged electrons show the conventional electric Hall effect. We find that [Formula: see text] is absent in the high-temperature paramagnetic state and develops upon entering the SL state in accordance with the growth of the short-range spin correlations, demonstrating that [Formula: see text] is a key signature of the elementary excitation formed in the SL state. These results suggest the emergence of nontrivial elementary excitations in the gapless SL state which feel the presence of fictitious magnetic flux, whose effective Lorentz force is found to be less than 1/100 of the force experienced by free electrons. PMID:27439874

  20. Theoretical study of spin-orbit and Coriolis coupling among the low-lying states of Rb2 and Cs2

    NASA Astrophysics Data System (ADS)

    Pazyuk, Elena A.; Revina, Elena I.; Stolyarov, Andrey V.

    2015-11-01

    The spin-orbit (SO) and angular (Coriolis) coupling matrix elements of rubidium and cesium dimers have been calculated between the states converging to the lowest three dissociation limits. The relevant quasi-relativistic matrix elements were evaluated for a wide range of internuclear distances and density grid in the basis of the spin-averaged wave functions corresponding to pure Hund's coupling case (a). Both shape and energy consistent small (9-electrons) effective core pseudopotentials were used to monitor a sensitivity of the matrix elements to the particular basis set. The dynamic correlation has been taken accounted by a large scale multi-reference configuration interaction method which was applied for only two valence electrons. The l-independent core-polarization potentials were employed to take into account the residual core-valence effect. The assessment of current accuracy of the present ab initio functions is discussed by a comparison with preceding calculations and their empirical counterparts.

  1. Fe-S Bonded Interactions Involving High and Low Spin State Divalent Fe Atoms

    NASA Astrophysics Data System (ADS)

    Gibbs, G. V.; Cox, D. F.; Rosso, K. M.; Ross, N. L.

    2006-12-01

    Bond critical point and local energy density properties together with the net atomic charges were generated for the theoretical electron density distributions, ρ(r), for a variety of Fe sulfide crystalline materials with high and low spin state divalent Fe atoms in octahedral coordination and high spin state divalent and trivalent Fe atoms in tetrahedral coordination. The value of the electron density, ρ(rc), and the Laplacian, ▽ 2ρ(rc), the local potential energy density, V(rc), and the local electronic energy density, H(rc), at bond critical points, (rc), each increases and the local kinetic energy density, G(rc), decreases as the coordination numbers of the Fe atoms decrease and the shared character of the Fe-S bonds is indicated to increase. The properties of the bonded interactions involving the octahedrally coordinated low spin state divalent Fe atoms in pyrite and marcasite depart substantially from those of the octahedrally coordinated high spin state divalent Fe atoms in troilite, symthite and greigite. The Fe-S bond lengths are shorter and the values of ρ(rc) and ▽ 2ρ(rc), are larger for pyrite and marcasite indicating that the accumulation and local concentration of ρ(r) in the vicinity of rc is greater than those involving the longer, high spin state Fe-S bonded interactions. The net atomic charges conferred on the Fe and S atoms in pyrite and marcasite are also smaller than those calculated for sulfides with high spin state octahedrally coordinate divalent Fe atoms. Collectively, the Fe-S bonded interactions are indicated to be intermediate in character on the basis of their bond indices with the low spin Fe-S bonds being more shared interactions than the high spin state bonded interactions. S-S bond paths exist between each of the surface S atoms of the adjacent layers of FeS6 octahedra in smythite, indicating that the neutral Fe3S4 layers are linked together by S-S bonded interactions. Such interactions not only exist between the S atoms on

  2. A projection gradient method for computing ground state of spin-2 Bose–Einstein condensates

    SciTech Connect

    Wang, Hanquan

    2014-10-01

    In this paper, a projection gradient method is presented for computing ground state of spin-2 Bose–Einstein condensates (BEC). We first propose the general projection gradient method for solving energy functional minimization problem under multiple constraints, in which the energy functional takes real functions as independent variables. We next extend the method to solve a similar problem, where the energy functional now takes complex functions as independent variables. We finally employ the method into finding the ground state of spin-2 BEC. The key of our method is: by constructing continuous gradient flows (CGFs), the ground state of spin-2 BEC can be computed as the steady state solution of such CGFs. We discretized the CGFs by a conservative finite difference method along with a proper way to deal with the nonlinear terms. We show that the numerical discretization is normalization and magnetization conservative and energy diminishing. Numerical results of the ground state and their energy of spin-2 BEC are reported to demonstrate the effectiveness of the numerical method.

  3. State diagram of magnetostatic coupling phase-locked spin-torque oscillators

    SciTech Connect

    Zhang, Mengwei; Wang, Longze; Wei, Dan; Gao, Kai-Zhong

    2015-05-07

    The state diagram of magnetostatic coupling phase-locked spin torque oscillator (STO) with perpendicular reference layer and planar field generation layer (FGL) is studied by the macrospin model and the micromagnetic model. The state diagrams of current densities are calculated under various external fields. The simulation shows that there are two phase-lock current density regions. In the phase-locked STOs in low current region I, the spin configuration of FGL is uniform; in high current region II, the spin configuration of FGL is highly nonuniform. In addition, the results with different STOs separation L{sub s} are compared, and the coupling between two STOs is largely decreased when L{sub s} is increased from 40 nm to 60 nm.

  4. Spin glass state and enhanced spiral phase in doped delafossite oxide CuCr O2

    NASA Astrophysics Data System (ADS)

    Yan, Z. R.; Qin, M. H.; Dong, S.; Zeng, M.; Lu, X. B.; Gao, X. S.; Liu, J.-M.

    2016-07-01

    In this paper, we study the doping effects on the magnetic states of CuCr O2 based on the classical frustrated spin model [13aa Lin et al., Phys. Rev. B 89, 220405(R) (2014), 10.1103/PhysRevB.89.220405]. Several experimental observations can be well reproduced by the Monte Carlo simulations of the modified spin models. Our paper suggests that the disorder induced by V/Al doping cooperating with the frustration in the system may contribute to the emergence of the spin glass state. Furthermore, the hole doping by M g2 + substituting C r3 + enhances the quantum fluctuations and bond disorder which modulate the biquadratic exchanges and in turn results in the promotion of the spiral phase, consistent with the experimental report.

  5. Frozen State and Spin Liquid Physics in Na4 Ir3 O8 : An NMR Study

    NASA Astrophysics Data System (ADS)

    Shockley, A. C.; Bert, F.; Orain, J.-C.; Okamoto, Y.; Mendels, P.

    2015-07-01

    Na4Ir3 O8 is a unique case of a hyperkagome 3D corner sharing triangular lattice that can be decorated with quantum spins. It has spurred a lot of theoretical interest as a spin liquid candidate. We present a comprehensive set of NMR data taken on both the 23Na and 17O sites. We show that disordered magnetic freezing of all Ir sites sets in below Tf˜7 K , well below J =300 K , with a drastic slowing down of fluctuations to a static state revealed by our T1 measurements. Above typically 2 Tf, physical properties are relevant to the spin liquid state induced by this exotic geometry. While the shift data show that the susceptibility levels off below 80 K, 1 /T1 has little variation from 300 K to 2 Tf. We discuss the implication of our results in the context of published experimental and theoretical work.

  6. Spin-Ice State of the Quantum Heisenberg Antiferromagnet on the Pyrochlore Lattice

    NASA Astrophysics Data System (ADS)

    Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris

    2016-04-01

    We study the low-temperature physics of the SU(2)-symmetric spin-1 /2 Heisenberg antiferromagnet on a pyrochlore lattice and find "fingerprint" evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are based on the results of bold diagrammatic Monte Carlo simulations, with good convergence of the skeleton series down to the temperature T /J =1 /6 . The identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for the static structure factor between the quantum Heisenberg, classical Heisenberg, and Ising models at all accessible temperatures, and the characteristic bowtie pattern with pinch points observed at T /J =1 /6 . The dynamic structure factor at real frequencies (obtained by the analytic continuation of numerical data) is consistent with diffusive spinon dynamics at the pinch points.

  7. Preformation probability inside α emitters having different ground state spin-parity than their daughters

    NASA Astrophysics Data System (ADS)

    Seif, W. M.; Botros, M. M.; Refaie, A. I.

    2015-10-01

    The ground state spin and parity of a daughter formed in a radioactive α emitter are expected to influence the preformation probability of the α and daughter clusters inside it. We investigate the α and daughter preformation probability inside odd-A and doubly odd radioactive nuclei when the daughter and parent are of different spin and/or parity. We consider only the ground state to ground state unfavored decays. This is to extract precise information about the effect of the difference in the spin-parity of the ground states of the involved nuclei far away from any influence from the excitation energy, if the decays are coming from isomeric states. The calculations are done for 161 α emitters, with 65 ≤Z ≤112 and 84 ≤N ≤173 , in the framework of the extended cluster model, with the Wentzel-Kramers-Brillouin penetrability and assault frequency. We used a Hamiltonian energy density scheme based on the Skyrme SLy4 interaction to compute the interaction potential. The α -plus-cluster preformation probability is extracted from the calculated decay width and the experimental half-life time. We discussed in detailed steps the effect of the angular momentum of the emitted α particle on the various physical quantities involved in the unfavored decay process and how it finally increases the half-life time. We found that if the ground state spin and/or parity of parent and daughter nuclei are different, then the preformation probability of the α cluster inside the parent is less than it would be if they had similar spin-parity. We modified the formula that gives the α preformation probability in terms of the numbers of protons and neutrons outside the shell closures of the parent, to account for this hindrance in the preformation probability for the unfavored decays between ground states.

  8. Investigation of high-spin states in 53Fe

    SciTech Connect

    du Rietz, R.; Williams, S.J.; Rudolph, D.; Ekman, J.; Fahlander,C.; Andreoiu, C.; Axiotis, M.; Bentley, M.A.; Carpenter, M.P.; Chandler,C.; Charity, R.J.; Clark, R.M.; Cromaz, M.; Dewald, A.; de Angelis, G.; Della Vedova, F.; Fallon, P.; Gadea, A.; Hammond, G.; Ideguchi, E.; Lenzi, S.M.; Macchiavelli, A.O.; Marginean, N.; Mineva, M.N.; Moller, O.; DNapoli, .R.; Nespolo, M.; Reviol, W.; Rusu, C.; Saha, B.; Sarantites,D.G.; Seweryniak, D.; Tonev, D.; Ur, C.A.

    2006-04-15

    The fusion-evaporation reactions 28Si(32S,1{alpha}2p1n)53Fe at 125 MeV and 24Mg(32S,2p1n)53Fe at a 95-MeV beam energy were used to investigate excited states in 53Fe. The combination of the Gammasphere Ge detector array and ancillary devices led to the construction of an extensive level scheme comprising some 90 transitions connecting 40 states. The lifetime of the yrast 25/2- state and upper limits for the lifetimes of a number of additional states were determined using the Cologne plunger device coupled to the GASP {gamma}-ray spectrometer. The experimental results are compared to large-scale shell-model calculations using different sets of two-body matrix elements. In particular, predictions on electromagnetic decay properties such as lifetimes, branching ratios, and mixing ratios are studied in detail.

  9. Spin Hamiltonian for the quantum Hall state in a ladder geometry

    NASA Astrophysics Data System (ADS)

    Kapit, E.; Luitel, P.; Schroeter, D. F.

    2006-02-01

    The first calculation of the true ground state of the parent Hamiltonian proposed by Laughlin [Laughlin, Ann. Phys. 191, 163 (1989)] for the m=2 fractional quantum Hall state on a torus is presented. Laughlin’s model is generalized to the case of a system in a ladder geometry and rewritten in terms of familiar spin-spin interactions, demonstrating that the model corresponds to a long-range Heisenberg Hamiltonian with an additional four-site interaction. The exact diagonalization of the Hamiltonian is performed to extract the energies, correlation functions, sublattice magnetization, and overlap with the quantum Hall state. Our results confirm the recent work showing that the model is not exact [Schroeter, Ann. Phys. 310, 155 (2004)] and also show it to be not without merit: the overlap between the quantum Hall (QH) state and exact ground state approaches the significant value of 0.83 in the limit that the ladder becomes infinitely long.

  10. Spin-Hamiltonian for the Quantum Hall State in a Ladder Geometry

    NASA Astrophysics Data System (ADS)

    Kapit, Eliot

    2005-03-01

    The first calculation of the true ground state of the parent-Hamiltonian proposed by Laughlin [R. B. Laughlin, Ann. Phys. 191, 163 (1989)] for the m=2 Fractional Quantum Hall state on a torus is presented. Laughlin's model is generalized to the case of a system in a ladder geometry and rewritten in terms of familiar spin-spin interactions, demonstrating that the model corresponds to a long-range Heisenberg Hamiltonian with an additional four-site interaction. The exact diagonalization of the Hamiltonian is performed to extract the energy, correlation functions, sub-lattice magnetization, and overlap with the Quantum Hall state. Our results confirm the recent work showing that the model is not exact [D. F. Schroeter, Ann. Phys. 310, 155 (2004)] and also show it to be not without merit: the overlap between the QH state and exact ground state approaches the significant value of 0.83 in the limit that the ladder becomes infinitely long.

  11. Observation of a highly spin-polarized topological surface state in GeBi2Te4

    NASA Astrophysics Data System (ADS)

    Okamoto, K.; Kuroda, K.; Miyahara, H.; Miyamoto, K.; Okuda, T.; Aliev, Z. S.; Babanly, M. B.; Amiraslanov, I. R.; Shimada, K.; Namatame, H.; Taniguchi, M.; Samorokov, D. A.; Menshchikova, T. V.; Chulkov, E. V.; Kimura, A.

    2012-11-01

    Spin polarization of a topological surface state for GeBi2Te4, the newly discovered three-dimensional topological insulator, has been studied by means of state-of-the-art spin- and angle-resolved photoemission spectroscopy. It has been revealed that the disorder in the crystal has a minor effect on the surface-state spin polarization, which is 70% near the Dirac point in the bulk energy gap region (˜180 meV). This finding promises not only to realize a highly spin-polarized surface-isolated transport but also to add functionality to its thermoelectric and thermomagnetic properties.

  12. Resonant Tunneling Spin Pump

    NASA Technical Reports Server (NTRS)

    Ting, David Z.

    2007-01-01

    The resonant tunneling spin pump is a proposed semiconductor device that would generate spin-polarized electron currents. The resonant tunneling spin pump would be a purely electrical device in the sense that it would not contain any magnetic material and would not rely on an applied magnetic field. Also, unlike prior sources of spin-polarized electron currents, the proposed device would not depend on a source of circularly polarized light. The proposed semiconductor electron-spin filters would exploit the Rashba effect, which can induce energy splitting in what would otherwise be degenerate quantum states, caused by a spin-orbit interaction in conjunction with a structural-inversion asymmetry in the presence of interfacial electric fields in a semiconductor heterostructure. The magnitude of the energy split is proportional to the electron wave number. Theoretical studies have suggested the possibility of devices in which electron energy states would be split by the Rashba effect and spin-polarized currents would be extracted by resonant quantum-mechanical tunneling.

  13. Probing iron spin state by optical absorption in laser-heated diamond anvil cell

    NASA Astrophysics Data System (ADS)

    Lobanov, S.; Goncharov, A. F.; Holtgrewe, N.; Lin, J. F.

    2015-12-01

    Pressure-induced spin-pairing transitions in iron-bearing minerals have been in the focus of geophysical studies1. Modern consensus is that iron spin state in the lower mantle is a complex function of crystal structure, composition, pressure, and temperature. Discontinuities in physical properties of lower mantle minerals have been revealed over the spin transition pressure range, but at room temperature. In this work, we have used a supercontinuum laser source and an intensified CCD camera to probe optical properties of siderite, FeCO3, and post-perovskite, Mg0.9Fe0.1SiO3, across the spin transition in laser-heated diamond anvil cell. Synchronously gating the CCD with the supercontinuum pulses (Fig. 1A) allowed diminishing thermal background to ~8.3*10-4. Utilizing the experimental setup we infer the spin state of ferrous iron in siderite at high pressure and temperature conditions (Fig. 1B). Similar behavior is observed for low spin ferric iron in post-perovskite at 130 GPa indicating that all iron in post-perovskite is high spin at lower mantle conditions. Also, our experimental setup holds promise for measuring radiative thermal conductivity of mantle minerals at relevant mantle conditions. Figure 1. (A) Timing of the optical absorption measurements at high temperature. (B) High temperature siderite absorption spectra at 45 GPa. Before heating and quenched after 1300 K spectra are shown in light and dark blue, respectively. Green and red curves are absorption spectra at 1200 K and 1300 K, respectively. Spectra shown in black represent room temperature absorption data on HS (43 GPa) and LS (45.5 GPa) siderite after Lobanov et al., 2015, shown for comparison.

  14. Reaching the ground state of a quantum spin glass using a zero-temperature quantum Monte Carlo method

    NASA Astrophysics Data System (ADS)

    Das, Arnab; Chakrabarti, Bikas K.

    2008-12-01

    Here we discuss the annealing behavior of an infinite-range ±J Ising spin glass in the presence of a transverse field using a zero-temperature quantum Monte Carlo method. Within the simulation scheme, we demonstrate that quantum annealing not only helps finding the ground state of a classical spin glass, but can also help simulating the ground state of a quantum spin glass, in particular, when the transverse field is low, much more efficiently.

  15. Reaching the ground state of a quantum spin glass using a zero-temperature quantum Monte Carlo method.

    PubMed

    Das, Arnab; Chakrabarti, Bikas K

    2008-12-01

    Here we discuss the annealing behavior of an infinite-range +/-J Ising spin glass in the presence of a transverse field using a zero-temperature quantum Monte Carlo method. Within the simulation scheme, we demonstrate that quantum annealing not only helps finding the ground state of a classical spin glass, but can also help simulating the ground state of a quantum spin glass, in particular, when the transverse field is low, much more efficiently. PMID:19256816

  16. Tunable self-assembled spin chains of strongly interacting cold atoms for demonstration of reliable quantum state transfer

    NASA Astrophysics Data System (ADS)

    Loft, N. J. S.; Marchukov, O. V.; Petrosyan, D.; Zinner, N. T.

    2016-04-01

    We have developed an efficient computational method to treat long, one-dimensional systems of strongly interacting atoms forming self-assembled spin chains. Such systems can be used to realize many spin chain model Hamiltonians tunable by the external confining potential. As a concrete demonstration, we consider quantum state transfer in a Heisenberg spin chain and we show how to determine the confining potential in order to obtain nearly perfect state transfer.

  17. Probing the population of the spin-orbit split levels in the actinide 5f states

    SciTech Connect

    Moore, K; der Laan, G v; Tobin, J; Chung, B; Wall, M; Schwartz, A

    2004-07-14

    Spin-orbit interaction in the 5f states is believed to strongly influence exotic behaviors observed in actinides metals and compounds. Understanding these interactions and how they relate to the actinide series is of considerable importance. To address this issue, the branching ratio of the white-line peaks of the N4,5 edges for the light actinide metals, {alpha}-Th, {alpha}-U, and {alpha}-Pu were recorded using electron energy-loss spectroscopy (EELS) in a transmission electron microscope (TEM) and synchrotron-radiation-based x-ray absorption spectroscopy (XAS). Using the spin-orbit sum rule and the branching ratios from both experimental spectra and many-electron atomic spectral calculations, accurate values of the spin-orbit interaction, and thus the relative occupation of the j = 5/2 and 7/2 levels, are determined for the actinide 5f states. Results show that the spin-orbit sum rule works very well with both EELS and XAS spectra, needing little or no correction. This is important, since the high spatial resolution of a TEM can be used to overcome the problems of single crystal growth often encountered with actinide metals, allowing acquisition of EELS spectra, and subsequent spin-orbit analysis, from nm-sized regions. The relative occupation numbers obtained by our method have been compared with recent theoretical results and show a good agreement in their trend.

  18. Quantum Transport of Spin-helical Dirac Fermion Topological Surface States in Topological Insulators

    NASA Astrophysics Data System (ADS)

    Chen, Yong P.

    Three-dimensional (3D) topological insulators (TI) are a novel class of electronic materials with topologically-nontrivial band structure such that the bulk is gapped and insulating yet the surface has topologically protected gapless conducting states. Such ``topological surface states'' (TSS) give helically spin polarized Dirac fermions, and offer a promising platform to realize various other novel physics such as topological magnetoelectric effects and Majorana fermions. However, it is often challenging to unambiguously access and study the transport properties of TSS in many practical TI materials due to non-negligible bulk conducting states. I will discuss our recent experiments on high-quality ``intrinsic'' TIs with insulating bulk and surface-dominated conduction that allow us to reveal a number of characteristic transport properties of spin-helical Dirac fermion topological surface states. We have observed, for example, a thickness-independent and surface-dominated conductance (even at room temperature) in exfoliated TI thin films and well-developed ``half-integer'' Dirac fermion quantum Hall effect (QHE) arising from TSS (observed up to 40K); fully-tunable ``two-species'' Dirac fermion QHE and other intriguing states in dual gated devices where both top and bottom surfaces can be independently controlled; current-induced helical spin-polarization detected by spin sensitive transport measurements using magnetic electrodes; and in TI nanoribbons, Shubnikov-de Hass (SdH) oscillations showing gate-tunable Berry phase and ultra-relativistic Dirac mass; and a ``half-integer'' Aharonov-Bohm effect (ABE) unique to the circumferentially quantized spin helical Dirac fermion surface state modes (sub-bands), with a gate-tunable conductance oscillation and alternation between the ``half-integer'' ABE and regular ABE periodic in fermi momentum. Such TIs and related devices may enable promising future applications in spintronics, thermoelectrics and various topological

  19. Design of defect spins in piezoelectric aluminum nitride for solid-state hybrid quantum technologies.

    PubMed

    Seo, Hosung; Govoni, Marco; Galli, Giulia

    2016-01-01

    Spin defects in wide-band gap semiconductors are promising systems for the realization of quantum bits, or qubits, in solid-state environments. To date, defect qubits have only been realized in materials with strong covalent bonds. Here, we introduce a strain-driven scheme to rationally design defect spins in functional ionic crystals, which may operate as potential qubits. In particular, using a combination of state-of-the-art ab-initio calculations based on hybrid density functional and many-body perturbation theory, we predicted that the negatively charged nitrogen vacancy center in piezoelectric aluminum nitride exhibits spin-triplet ground states under realistic uni- and bi-axial strain conditions; such states may be harnessed for the realization of qubits. The strain-driven strategy adopted here can be readily extended to a wide range of point defects in other wide-band gap semiconductors, paving the way to controlling the spin properties of defects in ionic systems for potential spintronic technologies. PMID:26876901

  20. Non-additive three-body interaction energies for H3 (quartet spin state)

    NASA Astrophysics Data System (ADS)

    Zhang, Z. C.; Allnatt, A. R.; Talman, James D.; Meath, William J.

    The results of an Unsold average energy calculation of the non-additive interaction energy for H3 (quartet spin state) are presented for equilateral triangular configurations. They are discussed in the context of the problems associated with the representation of non-additive energies for the interaction of closed-shell species.