Short Range Correlations in Nuclei at Large xbj through Inclusive Quasi-Elastic Electron Scattering
Ye, Zhihong
2013-12-01
The experiment, E08-014, in Hall-A at Jefferson Lab aims to study the short-range correlations (SRC) which are necessary to explain the nuclear strength absent in the mean field theory. The cross sections for 2H, 3He, 4He, 12C, 40Ca and 48Ca, were measured via inclusive quasi-elastic electron scattering from these nuclei in a Q2 range between 0.8 and 2.8 (GeV/c)^{2} for x>1. The cross section ratios of heavy nuclei to 2H were extracted to study two-nucleon SRC for 1
Quasi-elastic neutron scattering studies of protein dynamics
Rorschach, H.E.
1993-05-25
Results that shed new light on the study of protein dynamics were obtained by quasi-elastic neutron scattering. The triple axis instrument H-9 supplied by the cold source was used to perform a detailed study of the quasi-elastic spectrum and the Debye-Waller factor for trypsin in powder form, in solution, and in crystals. A preliminary study of myoglobin crystals was also done. A new way to view the results of quasi-elastic scattering experiments is sketched, and the data on trypsin are presented and analyze according to this new picture.
Improved Optics For Quasi-Elastic Light Scattering
NASA Technical Reports Server (NTRS)
Cheung, Harry Michael
1995-01-01
Improved optical train devised for use in light-scattering measurements of quasi-elastic light scattering (QELS) and laser spectroscopy. Measurements performed on solutions, microemulsions, micellular solutions, and colloidal dispersions. Simultaneous measurements of total intensity and fluctuations in total intensity of light scattered from sample at various angles provides data used, in conjunction with diffusion coefficients, to compute sizes of particles in sample.
Experimental study of quasi-elastic scattering of ultracold neutrons
NASA Astrophysics Data System (ADS)
Steyerl, A.; Yerozolimsky, B. G.; Serebrov, A. P.; Geltenbort, P.; Achiwa, N.; Pokotilovski, Yu. N.; Kwon, O.; Lasakov, M. S.; Krasnoshchokova, I. A.; Vasilyev, A. V.
2002-08-01
Ultracold neutrons (UCN) are lost from traps if they are quasi-elastically scattered from the wall with an energy gain sufficient to exceed the Fermi potential for the wall. Possible mechanisms of a quasi-elastic energy transfer are, for instance, scattering from hydrogen diffusing in an impurity surface layer or on surface waves at a liquid wall. Using two different experimental methods at the UCN source of the Institut Laue-Langevin we have investigated both the energy-gain and the energy-loss side of quasi-elastic UCN scattering on Fomblin grease coated walls. For Fomblin oil and similar new types of oil we report up-scattering data as a function of temperature and energy transfer. These low-temperature oils may be used in an improved measurement of the neutron lifetime, which requires extremely low wall reflection losses.
Quasi-elastic nuclear scattering at high energies
NASA Technical Reports Server (NTRS)
Cucinotta, Francis A.; Townsend, Lawrence W.; Wilson, John W.
1992-01-01
The quasi-elastic scattering of two nuclei is considered in the high-energy optical model. Energy loss and momentum transfer spectra for projectile ions are evaluated in terms of an inelastic multiple-scattering series corresponding to multiple knockout of target nucleons. The leading-order correction to the coherent projectile approximation is evaluated. Calculations are compared with experiments.
Two Photon Exchange in Quasi-elastic and Deep-inelastic Scattering
Averett, Todd D.; Katich, Joseph; Zhao Bo
2011-10-24
In this paper, I present an overview and preliminary results from three experiments at Jefferson Lab that were recently completed using a {sup 3}He gas target with polarization oriented normal to the scattering plane of unpolarized incident electrons. A target single spin asymmetry was formed by periodically flipping the direction of the target spin. In the reaction {up_arrow}{sup 3}He(e,e'), the Born contribution is expected to be zero, giving direct sensitivity to two photon exchange. This asymmetry was measured in the quasi-elastic and deep-inelastic regimes with 0.1 < Q{sup 2} < 1.0 GeV{sup 2}. The asymmetry is predicted to decrease by two-orders of magnitude for deep-inelastic versus quasi-elastic scattering. Preliminary results from these experiments will be presented.
Measurement of muon neutrino quasi-elastic scattering on carbon
Aguilar-Arevalo, A.A.; Bazarko, A.O.; Brice, S.J.; Brown, B.C.; Bugel, L.; Cao, J.; Coney, L.; Conrad, J.M.; Cox, D.C.; Curioni, A.; Djurcic, Z.; /Alabama U. /Bucknell U. /Cincinnati U. /Colorado U. /Columbia U. /Embry-Riddle Aeronautical U. /Fermilab /Indiana U. /Los Alamos /Louisiana State U. /Michigan U.
2007-06-01
Low energy (200 < E{sub v} < 2000 MeV) neutrino oscillation experiments, including MiniBooNE, require a model of charged current quasi-elastic (CCQE) neutrino interactions to predict signal samples. Using a high-statistics sample of muon neutrino CCQE events, MiniBooNE finds that a simple Fermi gas model, with appropriate adjustments, accurately characterizes the CCQE events observed in a carbon-based detector. The extracted parameters include an effective axial mass, M{sub A} = 1.23 {+-} 0.20 GeV, used to describe the four-momentum dependence of the axial-vector form factor of the nucleon; and a Pauli-suppression parameter, {kappa} = 1.019 {+-} 0.011.
Quasi-elastic light scattering from structured particles.
Chen, S H; Holz, M; Tartaglia, P
1977-01-01
We present a formulation by which the scattered field correlation function of a nonstationary structured particle can be calculated. Specifically, we consider the case of micron-size bacteria, where the Rayleigh- Gans-Debye approximation may be used to evaluate the correlation function. We show that the width of the intensity correlation spectrum (as measured, for example, by the photon correlation technique) exhibits I an oscillatory behavior which is characteristic of the interference pattern produced by the internal structure. Two cases are of interest: diffusion and motility are considered in detail, and some evidence of the predicted behavior is shown from the photon correlation measurement of E. coli bacteria. PMID:20168450
Rhodopsin Photoactivation Dynamics Revealed by Quasi-Elastic Neutron Scattering
NASA Astrophysics Data System (ADS)
Bhowmik, Debsindhu; Shrestha, Utsab; Perera, Suchhithranga M. C. D.; Chawla, Udeep; Mamontov, Eugene; Brown, Michael; Chu, Xiang-Qiang
2015-03-01
Rhodopsin is a G-protein-coupled receptor (GPCR) responsible for vision. During photoactivation, the chromophore retinal dissociates from protein yielding the opsin apoprotein. What are the changes in protein dynamics that occur during the photoactivation process? Here, we studied the microscopic dynamics of dark-state rhodopsin and the ligand-free opsin using quasielastic neutron scattering (QENS). The QENS technique tracks individual hydrogen atom motion because of the much higher neutron scattering cross-section of hydrogen than other atoms. We used protein with CHAPS detergent hydrated with heavy water. The activation of proteins is confirmed at low temperatures up to 300 K by mean-square displacement (MSD) analysis. The QENS experiments at temperatures ranging from 220 K to 300 K clearly indicate an increase in protein dynamic behavior with temperature. The relaxation time for the ligand-bound protein rhodopsin is faster compared to opsin, which can be correlated with the photoactivation. Moreover, the protein dynamics are orders of magnitude slower than the accompanying CHAPS detergent, which unlike protein, manifests localized motions.
A quasi-elastic light scattering study of smooth muscle myosin in the presence of ATP.
Wu, X; Blank, P S; Carlson, F D
1992-01-01
We have investigated the hydrodynamic properties of turkey gizzard smooth muscle myosin in solution using quasi-elastic light scattering (QELS). The effects of ionic strength (0.05-0.5 M KCl) and light chain phosphorylation on the conformational transition of myosin were examined in the presence of ATP at 20 degrees C. Cumulant analysis and light scattering models were used to describe the myosin system in solution. A nonlinear least squares fitting procedure was used to determine the model that best fits the data. The conformational transition of the myosin monomer from a folded form to an extended form was clearly demonstrated in a salt concentration range of 0.15-0.3 M KCl. Light chain phosphorylation regulates the transition and promotes unfolding of the myosin. These results agree with the findings obtained using sedimentation velocity and electron microscopy (Onishi and Wakabayashi, 1982; Trybus et al., 1982; Trybus and Lowey, 1984). In addition, we present evidence for polymeric myosin coexisting with the two monomeric myosin species over a salt concentration range from 0.05 to 0.5 M KCl. The size of the polymeric myosin varied with salt concentration. This observation supports the hypothesis that, in solution, a dynamic equilibrium exists between the two conformations of myosin monomer and filaments. PMID:1420864
Rorschach, H.E.
1993-05-25
Results that shed new light on the study of protein dynamics were obtained by quasi-elastic neutron scattering. The triple axis instrument H-9 supplied by the cold source was used to perform a detailed study of the quasi-elastic spectrum and the Debye-Waller factor for trypsin in powder form, in solution, and in crystals. A preliminary study of myoglobin crystals was also done. A new way to view the results of quasi-elastic scattering experiments is sketched, and the data on trypsin are presented and analyze according to this new picture.
Dorman, Mark Edward; /University Coll. London
2008-04-01
The Main Injector Neutrino Oscillation Search (MINOS) is a long baseline neutrino oscillation experiment based at the Fermi National Accelerator Laboratory (FNAL) in Chicago, Illinois. MINOS measures neutrino interactions in two large iron-scintillator tracking/sampling calorimeters; the Near Detector on-site at FNAL and the Far Detector located in the Soudan mine in northern Minnesota. The Near Detector has recorded a large number of neutrino interactions and this high statistics dataset can be used to make precision measurements of neutrino interaction cross sections. The cross section for charged-current quasi-elastic scattering has been measured by a number of previous experiments and these measurements disagree by up to 30%. A method to select a quasi-elastic enriched sample of neutrino interactions in the MINOS Near Detector is presented and a procedure to fit the kinematic distributions of this sample and extract the quasi-elastic cross section is introduced. The accuracy and robustness of the fitting procedure is studied using mock data and finally results from fits to the MINOS Near Detector data are presented.
Role of triple phonon excitations in large angle quasi-elastic scattering of very heavy mass systems
NASA Astrophysics Data System (ADS)
Zamrun, Muhammad Firihu
2016-07-01
We study the effect of multi-phonon excitations on large-angle quasi-elastic scattering of massive systems using the full order coupled-channels formalism. We especially investigate the role of triple phonon excitations of the target and projectile nuclei on the quasi-elastic scattering cross-section as well as the barrier distribution for 54Cr, 56Fe, 64Ni and 70Zn + 208Pb systems. It is shown that the calculations taken into account, the triple octupole phonon excitations of the target and triple quadrupole phonon excitations of the projectile for these systems can explain the experimental data of the quasi-elastic cross-section and the quasi-elastic barrier distribution. These results indicate that the coupled-channels formalism is still valid even for the very heavy mass systems.
NASA Astrophysics Data System (ADS)
Osti, N. C.; Coté, A.; Mamontov, E.; Ramirez-Cuesta, A.; Wesolowski, D. J.; Diallo, S. O.
2016-02-01
Understanding the molecular behavior of water in spatially restricted environments is key to better understanding its role in many biological, chemical and geological processes. Here we examine the translational diffusion of water confined to a variety of substrates, from flat surfaces to nanoporous media, in the context of a recently proposed universal scaling law (Chiavazzo 2014) [1]. Using over a dozen previous neutron scattering results, we test the validity of this law, evaluating separately the influence of the hydration amount, and the effects of the size and morphology of the confining medium. Additionally, we investigate the effects of changing instrument resolutions and fitting models on the applicability of this law. Finally, we perform quasi-elastic neutron scattering measurements on water confined inside nanoporous silica to further evaluate this predictive law, in the temperature range 250 ⩽ T ⩽ 290 K.
Fast proton hopping detection in ice I{sub h} by quasi-elastic neutron scattering.
Presiado, I.; Lal, J.; Mamontov, E.; Kolesnikov, A. I.; Huppert, D.
2011-01-01
Quasi-elastic neutron scattering was employed on samples of HCl-doped polycrystalline ice I{sub h}. The analysis of the scattering signal provides the excess proton hopping time, {tau}{sub hop}, in the temperature range of 140-195 K. The hopping time strongly depends on the temperature of the sample, and the activation energy of a hopping step is 17 kJ/mol. The values of {tau}{sub hop} of the current experiment are in good agreement with calculated values derived from previous photochemical experiments, in which we found that the proton hopping time at T > 242 K is on the order of 200 fs, roughly 10 times shorter than in liquid water at room temperature.
Fast Proton Hopping Detection in Ice Ih by Quasi-Elastic Neutron Scattering
Presiado, Itay; Lal, Jyotsana; Mamontov, Eugene; Kolesnikov, Alexander I; Huppert, Dan I
2011-01-01
Quasi-elastic neutron scattering was employed on samples of HCl-doped polycrystalline ice I{sub h}. The analysis of the scattering signal provides the excess proton hopping time, {tau}{sub hop}, in the temperature range of 140-195 K. The hopping time strongly depends on the temperature of the sample, and the activation energy of a hopping step is 17 kJ/mol. The values of {tau}{sub hop} of the current experiment are in good agreement with calculated values derived from previous photochemical experiments,(1) in which we found that the proton hopping time at T > 242 K is on the order of 200 fs, roughly 10 times shorter than in liquid water at room temperature.
Osti, Naresh C.; Mamontov, Eugene; Ramirez-cuesta, A.; Wesolowski, David J.; Diallo, S. O.
2015-12-10
Understanding the molecular behavior of water in spatially restricted environments is important to better understanding its role in many biological, chemical and geological processes. Here we examine the translational diffusion of water confined to a variety of substrates, from flat surfaces to nanoporous media, in the context of a recently proposed universal scaling law (Chiavazzo 2014) [1]. Using over a dozen previous neutron scattering results, we test the validity of this law, evaluating separately the influence of the hydration amount, and the effects of the size and morphology of the confining medium. Additionally, we investigate the effects of changing instrumentmore » resolutions and fitting models on the applicability of this law. Finally, we perform quasi-elastic neutron scattering measurements on water confined inside nanoporous silica to further evaluate this predictive law, in the temperature range 250≤T≤290 K.« less
Osti, Naresh C.; Mamontov, Eugene; Ramirez-cuesta, A.; Wesolowski, David J.; Diallo, S. O.
2015-12-10
Understanding the molecular behavior of water in spatially restricted environments is important to better understanding its role in many biological, chemical and geological processes. Here we examine the translational diffusion of water confined to a variety of substrates, from flat surfaces to nanoporous media, in the context of a recently proposed universal scaling law (Chiavazzo 2014) [1]. Using over a dozen previous neutron scattering results, we test the validity of this law, evaluating separately the influence of the hydration amount, and the effects of the size and morphology of the confining medium. Additionally, we investigate the effects of changing instrument resolutions and fitting models on the applicability of this law. Finally, we perform quasi-elastic neutron scattering measurements on water confined inside nanoporous silica to further evaluate this predictive law, in the temperature range 250≤T≤290 K.
Hydrogen Species Motion in Piezoelectrics: A Quasi-Elastic Neutron Scattering Study
Alvine, Kyle J.; Tyagi, Madhu; Brown, Craig; Udovic, Terrence J.; Jenkins, T. J.; Pitman, Stan G.
2012-03-05
Hydrogen is known to damage or degrade piezoelectric materials, at low pressure for ferroelectric random access memory applications, and at high pressure for hydrogen powered vehicle applications. The piezoelectric degradation is in part governed by the motion of hydrogen species within the piezoelectric materials. We present here Quasi-Elastic Neutron Scattering (QENS) measurements of the local hydrogen species motion within lead zirconate titanate (PZT) and barium titanate (BTO) on samples charged by gaseous exposure to high-pressure gaseous hydrogen {approx}17 MPa. Filter Analyzed Neutron Spectroscopy (FANS) studies of the hydrogen enhanced vibrational modes are presented as well. Results are discussed in context of theoretically predicted interstitial hydrogen lattice sites and compared to comparable bulk diffusion studies of hydrogen diffusion in lead zirconate titanate.
Vibrational lifetimes and friction in adsorbate motion determined from quasi-elastic scattering.
Lechner, Barbara A J; Hedgeland, Holly; Jardine, Andrew P; Allison, William; Hinch, B J; Ellis, John
2015-09-14
The vibrational excitation of molecules adsorbed on a surface is typically probed by spectroscopic techniques such as infrared or Raman spectroscopy. In the present article we demonstrate an alternative method to determine vibrational lifetimes of adsorbate molecules using quasi-elastic helium atom scattering (QHAS). As a probe of diffusive motion of molecules on surfaces QHAS is well established. Here, we demonstrate that QHAS can also be used to probe the vibrational lifetime of a molecule in its adsorption well. Measurements of cyclopentadienyl, C5H5, on Cu(111) allow us to distinguish two substrate phonon modes as well as two molecular vibrational modes, perpendicular and parallel to the surface. We further find that the dephasing of the vibrational motion corresponds to the friction determined in previous diffusion measurements. PMID:26204093
Quasi elastic and inelastic neutron scattering study of vitamin C aqueous solutions
NASA Astrophysics Data System (ADS)
Migliardo, F.; Branca, C.; Magazù, S.; Migliardo, P.; Coppolino, S.; Villari, A.; Micali, N.
2002-02-01
In this paper, new results obtained by quasi elastic and inelastic neutron scattering experiments performed on vitamin C ( L-ascorbic acid)/H 2O mixtures are reported. The data analysis of the QENS measurements, by a separation of the diffusive dynamics of hydrated L-ascorbic acid from that of water, furnishes quantitative evidences of a random jump diffusion motion of vitamin C and shows that the water dynamics is strongly affected by the presence of L-ascorbic acid. Concerning the INS experiment, we are able, through the behaviour of neutron spectra across the glass transition temperature ( T g≈233 K for the vitamin C/water system), to collocate the investigated system in the Angell “strong-fragile” scheme.
Analysis of a quasi-elastic laser scattering spectrum using the maximum entropy method.
Tsuyumoto, Isao
2007-12-01
We have applied the maximum entropy method (MEM) to the analysis of quasi-elastic laser scattering (QELS) spectra and have established a technique for determining capillary wave frequencies with a higher time resolution than that of the conventional procedure. Although the QELS method has an advantage in time resolution over mechanical methods, it requires the averaging of at least 20-100 power spectra for determining capillary wave frequencies. We find that the MEM analysis markedly improves the S/N ratio of the power spectra, and that averaging the spectra is not necessary for determining the capillary wave frequency, i.e., it can be estimated from one power spectrum. The time resolution of the QELS attains the theoretical limit by using MEM analysis. PMID:18071233
NASA Astrophysics Data System (ADS)
Sargsyan, V. V.; Adamian, G. G.; Antonenko, N. V.; Diaz-Torres, A.; Gomes, P. R. S.; Lenske, H.
2015-11-01
We present a simple method to derive breakup probabilities of weakly bound nuclei by measuring only elastic (or quasi-elastic) scattering for the system under investigation and a similar tightly bound system. When transfer followed by breakup is an important process, one can derive only the sum of breakup and transfer probabilities.
Quasi-elastic neutron scattering studies of the slow dynamics of supercooled and glassy aspirin
NASA Astrophysics Data System (ADS)
Zhang, Yang; Tyagi, Madhusudan; Mamontov, Eugene; Chen, Sow-Hsin
2012-02-01
Aspirin, also known as acetylsalicylic acid (ASA), is not only a wonderful drug, but also a good glass former. Therefore, it serves as an important molecular system to study the near-arrest and arrested phenomena. In this paper, a high-resolution quasi-elastic neutron scattering (QENS) technique is used to investigate the slow dynamics of supercooled liquid and glassy aspirin from 410 down to 350 K. The measured QENS spectra can be analyzed with a stretched exponential model. We find that (i) the stretched exponent β(Q) is independent of the wavevector transfer Q in the measured Q range and (ii) the structural relaxation time τ(Q) follows a power-law dependence on Q. Consequently, the Q-independent structural relaxation time τ0 can be extracted for each temperature to characterize the slow dynamics of aspirin. The temperature dependence of τ0 can be fitted with the mode-coupling power law, the Vogel-Fulcher-Tammann equation and a universal equation for fragile glass forming liquids recently proposed by Tokuyama in the measured temperature range. The calculated dynamic response function χT(Q, t) using the experimentally determined self-intermediate scattering function of the hydrogen atoms of aspirin shows direct evidence of the enhanced dynamic fluctuations as the aspirin is increasingly supercooled, in agreement with the fixed-time mean squared displacement langx2rang and the non-Gaussian parameter α2 extracted from the elastic scattering.
Quasi-Elastic Neutron Scattering Studies of the Slow Dynamics of Supercooled and Glassy Aspirin
Zhang, Yang; Tyagi, M.; Mamontov, Eugene; Chen, Sow-hsin H
2011-01-01
Aspirin, also known as acetylsalicylic acid (ASA), is not only a wonderful drug, but also a good glass former. Therefore, it serves as an important molecular system to study the near-arrest and arrested phenomena. In this paper, a high-resolution quasi-elastic neutron scattering (QENS) technique is used to investigate the slow dynamics of supercooled liquid and glassy aspirin from 410 K down to 350 K. The measured QENS spectra can be analyzed with a stretched exponential model. We find that (i) the stretched exponent (Q) is independent of the wave vector transfer Q in the measured Q-range, and (ii) the structural relaxation time (Q) follows a power law dependence on Q. Consequently, the Q-independent structural relaxation time 0 can be extracted for each temperature to characterize the slow dynamics of aspirin. The temperature dependence of 0 can be fitted with the mode coupling power law, the Vogel-Fulcher-Tammann equation and a universal equation for fragile glass forming liquids recently proposed by M. Tokuyama in the measured temperature range. The calculated dynamic response function T(Q,t) using the experimentally determined self-intermediate scattering function of the hydrogen atoms of aspirin shows a direct evidence of the enhanced dynamic fluctuations as the aspirin is increasingly supercooled, in agreement with the fixed-time mean squared displacement x2 and non-Gaussian parameter 2 extracted from the elastic scattering.
Quasi-elastic light scattering in betaine calcium chloride dihydrate (BCCD)
NASA Astrophysics Data System (ADS)
Schmitt-Lewen, M.; Schaack, G.
1999-12-01
We report measurements of the temperature (40 Kicons/Journals/Common/le" ALT="le" ALIGN="TOP"/> T icons/Journals/Common/le" ALT="le" ALIGN="TOP"/>200 K) and polarization (z(yy)x,z(xz)x) dependence of the integrated intensities of quasi-elastically scattered laser light (icons/Journals/Common/lambda" ALT="lambda" ALIGN="TOP"/> = 514.5 nm) in a wavenumber interval of 0+/-3 cm-1 around the Rayleigh line at the different phase transitions in single crystals of BCCD. Large anomalies (central peaks) are observed at the transitions into the ferroelectric, the various commensurate (c,c´), and the incommensurate phases. The widths of the anomalies on the temperature scale are large in the regions of quasi-harmonic modulation of the structure, but narrow and distinct in the region of square-wave modulation in the solitonic phase of BCCD, where also unusual shapes on the T-axis are observed. The scattering phenomena at low temperatures are interpreted hypothetically as due to fluctuations caused by the formation or rearrangement of domain walls (solitons) in the lattice near the transitions between commensurate phases and by the variation in soliton density. The cicons/Journals/Common/leftrightarrow" ALT="leftrightarrow" ALIGN="TOP"/>c´ transitions are of the order-disorder type.
Zamrun, Muhammad F.; Kasim, Hasan Abu
2011-03-30
We study the large angle quasi-elastic scattering of {sup 54}Cr+{sup 208}Pb system in terms of the full-order coupled-channels formalism. We especially investigate the role of single, double and triple phonon excitations on quasi-elastic scattering cross section as well as quasi-elastic barrier distribution of this system for which the experimental data have been measured. It is shown that the triple phonon excitations both in {sup 54}Cr and {sup 208}Pb nuclei seem to be needed by the present coupled-channels calculations in order to reproduce the experimental data of quasi-elastic cross section and barrier distribution for the {sup 54}Cr+{sup 208}Pb system. We also show that the standard value of the surface diffuseness parameter for the nuclear potential a = 0.63 fm, is preferred by the experimental quasi-elastic scattering data for this system.
A Quasi-Elastic Neutron Scattering Study of the Dynamics of Electrically Constrained Water.
Fuchs, Elmar C; Bitschnau, Brigitte; Wexler, Adam D; Woisetschläger, Jakob; Freund, Friedemann T
2015-12-31
We have measured the quasi-elastic neutron scattering (QENS) of an electrohydrodynamic liquid bridge formed between two beakers of pure water when a high voltage is applied, a setup allowing to investigate water under high-voltage without high currents. From this experiment two proton populations were distinguished: one consisting of protons strongly bound to oxygen atoms (immobile population, elastic component) and a second one of quasi-free protons (mobile population, inelastic component) both detected by QENS. The diffusion coefficient of the quasi-free protons was found to be D = (26 ± 10) × 10(-5) cm(2) s(-1) with a jump length lav ∼ 3 Å and an average residence time of τ0 = 0.55 ± 0.08 ps. The associated proton mobility in the proton channel of the bridge is ∼9.34 × 10(-7) m(2) V(-1) s(-1), twice as fast as diffusion-based proton mobility in bulk water. It also matches the so-called electrohydrodynamic or "apparent" charge mobility, an experimental quantity which so far has lacked molecular interpretation. These results further corroborate the proton channel model for liquid water under high voltage and give new insights into the molecular mechanisms behind electrohydrodynamic charge transport phenomena and delocalization of protons in liquid water. PMID:26643863
Molecular dynamics force-field refinement against quasi-elastic neutron scattering data
Borreguero Calvo, Jose M.; Lynch, Vickie E.
2015-11-23
Quasi-elastic neutron scattering (QENS) is one of the experimental techniques of choice for probing the dynamics at length and time scales that are also in the realm of full-atom molecular dynamics (MD) simulations. This overlap enables extension of current fitting methods that use time-independent equilibrium measurements to new methods fitting against dynamics data. We present an algorithm that fits simulation-derived incoherent dynamical structure factors against QENS data probing the diffusive dynamics of the system. We showcase the difficulties inherent to this type of fitting problem, namely, the disparity between simulation and experiment environment, as well as limitations in the simulationmore » due to incomplete sampling of phase space. We discuss a methodology to overcome these difficulties and apply it to a set of full-atom MD simulations for the purpose of refining the force-field parameter governing the activation energy of methyl rotation in the octa-methyl polyhedral oligomeric silsesquioxane molecule. Our optimal simulated activation energy agrees with the experimentally derived value up to a 5% difference, well within experimental error. We believe the method will find applicability to other types of diffusive motions and other representation of the systems such as coarse-grain models where empirical fitting is essential. In addition, the refinement method can be extended to the coherent dynamic structure factor with no additional effort.« less
Molecular dynamics force-field refinement against quasi-elastic neutron scattering data
Borreguero Calvo, Jose M.; Lynch, Vickie E.
2015-11-23
Quasi-elastic neutron scattering (QENS) is one of the experimental techniques of choice for probing the dynamics at length and time scales that are also in the realm of full-atom molecular dynamics (MD) simulations. This overlap enables extension of current fitting methods that use time-independent equilibrium measurements to new methods fitting against dynamics data. We present an algorithm that fits simulation-derived incoherent dynamical structure factors against QENS data probing the diffusive dynamics of the system. We showcase the difficulties inherent to this type of fitting problem, namely, the disparity between simulation and experiment environment, as well as limitations in the simulation due to incomplete sampling of phase space. We discuss a methodology to overcome these difficulties and apply it to a set of full-atom MD simulations for the purpose of refining the force-field parameter governing the activation energy of methyl rotation in the octa-methyl polyhedral oligomeric silsesquioxane molecule. Our optimal simulated activation energy agrees with the experimentally derived value up to a 5% difference, well within experimental error. We believe the method will find applicability to other types of diffusive motions and other representation of the systems such as coarse-grain models where empirical fitting is essential. In addition, the refinement method can be extended to the coherent dynamic structure factor with no additional effort.
Trantham, E C; Rorschach, H E; Clegg, J S; Hazlewood, C F; Nicklow, R M; Wakabayashi, N
1984-01-01
Results have been obtained on the quasi-elastic spectra of neutrons scattered from pure water, a 20% agarose gel (hydration four grams H2O per gram of dry solid) and cysts of the brine shrimp Artemia for hydrations between 0.10 and 1.2 grams H2O per gram of dry solids. The spectra were interpreted using a two-component model that included contributions from the covalently bonded protons and the hydration water, and a mobile water fraction. The mobile fraction was described by a jump-diffusion correlation function for the translation motion and a simple diffusive orientational correlation function. The results for the line widths gamma (Q2) for pure water were in good agreement with previous measurements. The agarose results were consistent with NMR measurements that show a slightly reduced translational diffusion for the mobile water fraction. The Artemia results show that the translational diffusion coefficient of the mobile water fraction was greatly reduced from that of pure water. The line width was determined mainly by the rotational motion, which was also substantially reduced from the pure water value as determined from dielectric relaxation studies. The translational and rotational diffusion parameters were consistent with the NMR measurements of diffusion and relaxation. Values for the hydration fraction and the mean square thermal displacement [u2] as determined from the Q-dependence of the line areas were also obtained. PMID:6733243
Energy dissipation in heavy systems: the transition from quasi-elastic to deep-inelastic scattering
Rehm, K.E.; van den Berg, A.; Kolata, J.J.; Kovar, D.G.; Kutschera, W.; Rosner, G.; Stephans, G.S.F.; Yntema, J.L.; Lee, L.L.
1984-01-01
The interaction of medium mass projectiles (A = 28 - 64) with /sup 208/Pb has been studied using a split-pole spectrograph which allows single mass and charge identification. The reaction process in all systems studied so far is dominated by quasi-elastic neutron transfer reactions, especially at incident energies in the vicinity of the Coulomb barrier. In addition to the quasi-elastic component deep inelastic contributions are present in all reaction channels. The good mass and charge separation allows to generate Wilczynski plots for individual channels; for the system /sup 48/Ti + /sup 208/Pb we observe that the transition between the quasi-elastic and deep-inelastic reactions occurs around Q = -(30 to 35) MeV.
Study of the Quasi-Elastic Scattering in the NOvA Detector Prototype
Betancourt, Minerba
2013-06-01
NOvA is a 810 km long base-line neutrino oscillation experiment with two detectors (far 14 KTon and near detector 300 Ton) currently being installed in the NUMI o -axis neutrino beam produced at Fermilab. A 222 Ton prototype NOvA detector (NDOS) was built and operated in the neutrino beam for over a year to understand the response of the detector and its construction. The goal of this thesis is to study the muon neutrino interaction data collected in this test, specifically the identification of quasi-elastic charged-current interactions and measure the behavior of the quasi-elastic muon neutrino cross section.
Study of quasi-elastic scattering in the NOνA near detector prototype
Betancourt, M.
2015-05-15
NOvA is a 14 kTon long-baseline neutrino oscillation experiment currently being installed in the NuMI off-axis neutrino beam produced at Fermilab. A 222 Ton prototype NOνA detector was built and operated in the neutrino beam for over a year to understand the response of the detector and its construction. Muon neutrino interaction data collected in this test are being analyzed to identify quasi-elastic charged-current interactions and measure the behavior of the quasi-elastic muon neutrino cross section.
Anti-Neutrino Charged Current Quasi-Elastic Scattering in MINER$\
Chvojka, Jesse John
2012-01-01
The phenomenon of neutrino oscillation is becoming increasingly understood with results from accelerator-based and reactor-based experiments, but unanswered questions remain. The proper ordering of the neutrino mass eigenstates that compose the neutrino avor eigenstates is not completely known. We have yet to detect CP violation in neutrino mixing, which if present could help explain the asymmetry between matter and anti-matter in the universe. We also have not resolved whether sterile neutrinos, which do not interact in any Standard Model interaction, exist. Accelerator-based experiments appear to be the most promising candidates for resolving these questions; however, the ability of present and future experiments to provide answers is likely to be limited by systematic errors. A significant source of this systematic error comes from limitations in our knowledge of neutrino-nucleus interactions. Errors on cross-sections for such interactions are large, existing data is sometimes contradictory, and knowledge of nuclear effects is incomplete. One type of neutrino interaction of particular interest is charged current quasi-elastic (CCQE) scattering, which yields a final state consisting of a charged lepton and nucleon. This process, which is the dominant interaction near energies of 1 GeV, is of great utility to neutrino oscillation experiments since the incoming neutrino energy and the square of the momentum transferred to the final state nucleon, Q^{2}, can be reconstructed using the final state lepton kinematics. To address the uncertainty in our knowledge of neutrino interactions, many experiments have begun making dedicated measurements. In particular, the MINER A experiment is studying neutrino-nucleus interactions in the few GeV region. MINERvA is a fine-grained, high precision, high statistics neutrino scattering experiment that will greatly improve our understanding of neutrino cross-sections and nuclear effects that affect the final state particles
Quasi-elastic Scattering Measurements in the {sup 6,7}Li+{sup 144}Sm Systems
Capurro, O. A.; Arazi, A.; Fernandez Niello, J. O.; Figueira, J. M.; Marti, G. V.; Martinez Heimann, D.; Negri, A. E.; Pacheco, A. J.; Monteiro, D. S.; Otomar, D. R.; Gomes, P. R. S.
2009-06-03
In the present work, results of measurements of quasi-elastic scattering cross sections using a silicon-telescope detector at backward angles are reported. They allowed us to deduce fusion barrier distributions from the first derivative of the corresponding excitation function (-d(d{sigma}{sub qes}/d{sigma}{sub Rut})/dE). We report data for the systems {sup 6,7}Li on {sup 144}Sm which are characterized by loosely bound projectiles onto a closed neutron shell target. The experimental excitation functions and the associated barrier distributions are compared for both systems.
Quasi-Elastic Neutron Scattering (QENS) Studies of Hydrogen Dynamics for Nano-Confined NaAlH4
NASA Astrophysics Data System (ADS)
Dobbins, Tabbetha; Narasegowda, Shathabish; Brown, Craig; Tyagi, Madhusudan; Jenkins, Timothy
The hydrogen dynamics of nano-confined sodium alanate (NaAlH4) has been studied using quasi-elastic neutron scattering (QENS). Results indicate thermodynamic destabilization is responsible for reduced desorption temperatures of NaAlH4 upon confinement within the nanopores of a metal organic framework (MOF). Both the bulk (microscale) NaAlH4 and the nanoconfined NaAlH4 data were fitted to re-orientation models which yielded corresponding percent mobile hydrogen and jump lengths. The jump lengths calculated from the nano-NaAlH4 were ~2.5 Å, and in conformity with those jump lengths determined for bulk NaAlH4 of ~2.3 Å. As much as 18 % of the hydrogen atoms were estimated to be mobile in the nano-NaAlH4 sample even at relatively low temperatures of 350 K. In contrast, bulk NaAlH4 shows less than 7 % mobile H-atoms even at higher temperatures of ~450 K. The activation energy for the long range is 3.1meV. Quasi-Elastic Neutron Scattering (QENS) Studies of Hydrogen Dynamics for Nano-Confined NaAlH4.
Wolcott, Jeremy
2016-01-01
Appearance-type neutrino oscillation experiments, which observe the transition from muon neutrinos to electron neutrinos, promise to help answer some of the fundamental questions surrounding physics in the post-Standard-Model era. Because they wish to observe the interactions of electron neutrinos in their detectors, and because the power of current results is typically limited by their systematic uncertainties, these experiments require precise estimates of the cross-section for electron neutrino interactions. Of particular interest is the charged-current quasi-elastic (CCQE) process, which gures signi cantly in the composition of the reactions observed at the far detector. However, no experimental measurements of this crosssection currently exist for electron neutrinos; instead, current experiments typically work from the abundance of muon neutrino CCQE cross-section data and apply corrections from theoretical arguments to obtain a prediction for electron neutrinos. Veri cation of these predictions is challenging due to the di culty of constructing an electron neutrino beam, but the advent of modern high-intensity muon neutrino beams|together with the percent-level electron neutrino impurity inherent in these beams| nally presents the opportunity to make such a measurement. We report herein the rst-ever measurement of a cross-section for an exclusive state in electron neutrino scattering, which was made using the MINER A detector in the NuMI neutrino beam at Fermilab. We present the electron neutrino CCQE di erential cross-sections, which are averaged over neutrinos of energies 1-10 GeV (with mean energy of about 3 GeV), in terms of various kinematic variables: nal-state electron angle, nal-state electron energy, and the square of the fourmomentum transferred to the nucleus by the neutrino , Q^{2}. We also provide a total cross-section vs. neutrino energy. While our measurement of this process is found to be in agreement with the predictions of the GENIE
Takahashi, Yoshihiro; Nakamura, Kensaku; Osada, Minoru; Fujiwara, Takumi
2012-01-01
Inelastic light scattering has been utilized for examining the structure of glass and its relaxation. However, the quasi-elastic-light-scattering (QLS) phenomenon has not been addressed in much detail. In this study, we observed pronounced QLS-intensity variations in two temperature domains—supercooled liquid (SCL) state (α-relaxation regime) and below the glass-transition temperature (β-relaxation regime)—in niobium-oxide (Nb2O5)-rich glass. These variations may be interpreted on the basis of the concept of ferroelectric and ion-conducting phases. It was suggested that the observed QLS originates as a result of the polarization fluctuation of NbO6 units, which is due to the dynamics of the nanometric phase separation in the SCL phase (α-regime), and the fluctuation due to the migration/hopping of conductible ions that are localized in the vicinity of the NbO6 units (β-regime). PMID:23056906
NASA Astrophysics Data System (ADS)
Gouesbet, G.; Grehan, G.
1981-06-01
Advances in quasi-elastic scattering of light are studied, and the theoretical analysis includes: (1) a generalized Lorenz-Mie theory (GLMT), describing the quasi-elastic linear scattering of light; (2) a computer program using the Lentz algorithm to compute ratios of Bessel functions; (3) a comparative analysis of the GLMT and geometrical optics; and (4) a discussion of new monotonic relationships between scattered powers and the sizes of scatter centers. The theoretical results are applied to the experimental study which attempts to measure simultaneously the diameter and velocity of individual particles embedded in laminar and turbulent two-phase flows, illuminated by a laser beam. Results show a satisfactory agreement with the theoretical predictions, and it is concluded that simultaneous velocimetry of single particles can be achieved by superimposing on the sizing probe a classical LDV control volume.
Trantham, E.C.; Rorschach, H.E.; Clegg, J.S.; Hazlewood, C.F.; Nicklow, R.M.; Wakabayashi, N.
1984-05-01
Results have been obtained on the quasi-elastic spectra of neutrons scattered from pure water, 20% agarose gel (hydration four grams H/sub 2/O per gram of dry solid) and cysts of the brine shrimp Artemia for hydrations between 0.10 and 1.2 grams H/sub 2/O per gram of dry solids. The spectra were interpreted using a two-component model that included contributions from the covalently bonded protons and the hydration water, and a mobile water fraction. The mobile fraction was described by a jump-diffusion correlation function for the translation motion and a simple diffusive orientational correlation function. The results for the line widths ..gamma..(Q/sup 2/) for pure water were in good agreement with previous measurements. The agarose results were consistent with NMR measurements that show a slightly reduced translational diffusion for the mobile water fraction. The Artemia results show that the translational diffusion coefficient of the mobile water fraction was greatly reduced from that of pure water. The line width was determined mainly by the rotational motion, which was also substantially reduced from the pure water value as determined from dielectric relaxation studies. The translational and rotational diffusion parameters were consistent with the NMR measurements of diffusion and relaxation. Values for the hydration fraction and the mean square thermal displacement as determined from the Q-dependence of line areas were also obtained.
Patrick, Cheryl
2016-01-01
Next-generation neutrino oscillation experiments, such as DUNE and Hyper-Kamiokande, hope to measure charge-parity (CP) violation in the lepton sector. In order to do this, they must dramatically reduce their current levels of uncertainty, particularly those due to neutrino-nucleus interaction models. As CP violation is a measure of the difference between the oscillation properties of neutrinos and antineutrinos, data about how the less-studied antineutrinos interact is especially valuable. We present the MINERvA experiment's first double-differential scattering cross sections for antineutrinos on scintillator, in the few-GeV range relevant to experiments such as DUNE and NOvA. We also present total antineutrino-scintillator quasi-elastic cross sections as a function of energy, which we compare to measurements from previous experiments. As well as being useful to help reduce oscillation experiments' uncertainty, our data can also be used to study the prevalence of various cor relation and final-state interaction effects within the nucleus. We compare to models produced by different model generators, and are able to draw first conclusions about the predictions of these models.
Ahmed, A I; Feeney, R E; Osuga, D T; Yeh, Y
1975-05-10
A quasi-elastic light-scattering technique was used to study the hydrodynamic conformations of antifreeze glycoproteins from an Antarctic fish. Antifreeze glycoprotein is composed of repeating units of Ala-Ala-Thr, with each threonine O-linked to a disaccharide, and it exists as several polymers of different numbers of this repeating unit. Molecular weights of the two major active polymers are 10,500 and 17,500 by such methods as centrifugation and osmotic pressure, but smaller than 20 by freezing-point depression. Translational diffusion coefficients at 20 degrees were 8.35 times 10-7 cm2 s-1 and 6.15 times 10-7 cm2 s-1 for the M-r-10,500 and 17,500 polymers, respectively. Measurements at -0.2 degrees in the presence of ice crystals did not indicate any conformational changes that might be related to the lowering of the freezing temperature. Lowering the temperature of these glycoprotein solutions close to temperatures of freezing caused a decrease in the effective hydrodynamic radius of both active and inactive glycoprotein components. PMID:1168194
Quasi-elastic light-scattering studies of single skeletal muscle fibers.
Haskell, R C; Carlson, F D
1981-01-01
Measurements were made of the intensity autocorrelation function, g(2)[tau], of light scattered from intact frog muscle fibers. During the tension plateau of an isometric tenanus, scattered field statistics were approximately Gaussian and intensity fluctuations were quasi-stationary. The half time, tau 1/2, for the decay of g(2)[tau] was typically 70 ms at a scattering angle of 30 degrees. The decay rate, 1/tau 1/2, of g(2)[tau] varied roughly linearly with the projection of the scattering vector on the fiber axis. 1/tau 1/2 was greater during the tension creep phase of tetani of highly stretched fibers, but was roughly independent of sarcomere length during the tension plateau. g(2)[tau] measured during rest or on diffraction pattern maxima during isometric contraction were flat with low amplitudes. These results are consistent with a model of a 200-mu m segment of an isometrically contracting fiber in which scattering material possesses relative axial velocities of 1-2 mu m/s accompanied by relative axial displacements greater than 0.1 mu m. The slow (1-2 mu m/s) motion of one portion of the fiber relative to another observed under the microscope (500X) during isometric contraction is consistent with the light-scattering results. Structural fluctuations on the scale of the myofibrillar sarcomere which may arise from asynchronous cycling of cross-bridges must involve relative axial velocities less than 3 mu m/s or relative axial displacements less than 0.05 mu m. PMID:6974014
NASA Astrophysics Data System (ADS)
Pantatosaki, Evangelia; Jobic, Hervé; Kolokolov, Daniil I.; Karmakar, Shilpi; Biniwale, Rajesh; Papadopoulos, George K.
2013-01-01
The problem of simulating processes involving equilibria and dynamics of guest sorbates within zeolitic imidazolate frameworks (ZIF) by means of molecular dynamics (MD) computer experiments is of growing importance because of the promising role of ZIFs as molecular "traps" for clean energy applications. A key issue for validating such an atomistic modeling attempt is the possibility of comparing the MD results, with real experiments being able to capture analogous space and time scales to the ones pertained to the computer experiments. In the present study, this prerequisite is fulfilled through the quasi-elastic neutron scattering technique (QENS) for measuring self-diffusivity, by elaborating the incoherent scattering signal of hydrogen nuclei. QENS and MD experiments were performed in parallel to probe the hydrogen motion, for the first time in ZIF members. The predicted and measured dynamics behaviors show considerable concentration variation of the hydrogen self-diffusion coefficient in the two topologically different ZIF pore networks of this study, the ZIF-3 and ZIF-8. Modeling options such as the flexibility of the entire matrix versus a rigid framework version, the mobility of the imidazolate ligand, and the inclusion of quantum mechanical effects in the potential functions were examined in detail for the sorption thermodynamics and kinetics of hydrogen and also of deuterium, by employing MD combined with Widom averaging towards studying phase equilibria. The latter methodology ensures a rigorous and efficient way for post-processing the dynamics trajectory, thereby avoiding stochastic moves via Monte Carlo simulation, over the large number of configurational degrees of freedom a nonrigid framework encompasses.
Pantatosaki, Evangelia; Jobic, Hervé; Kolokolov, Daniil I; Karmakar, Shilpi; Biniwale, Rajesh; Papadopoulos, George K
2013-01-21
The problem of simulating processes involving equilibria and dynamics of guest sorbates within zeolitic imidazolate frameworks (ZIF) by means of molecular dynamics (MD) computer experiments is of growing importance because of the promising role of ZIFs as molecular "traps" for clean energy applications. A key issue for validating such an atomistic modeling attempt is the possibility of comparing the MD results, with real experiments being able to capture analogous space and time scales to the ones pertained to the computer experiments. In the present study, this prerequisite is fulfilled through the quasi-elastic neutron scattering technique (QENS) for measuring self-diffusivity, by elaborating the incoherent scattering signal of hydrogen nuclei. QENS and MD experiments were performed in parallel to probe the hydrogen motion, for the first time in ZIF members. The predicted and measured dynamics behaviors show considerable concentration variation of the hydrogen self-diffusion coefficient in the two topologically different ZIF pore networks of this study, the ZIF-3 and ZIF-8. Modeling options such as the flexibility of the entire matrix versus a rigid framework version, the mobility of the imidazolate ligand, and the inclusion of quantum mechanical effects in the potential functions were examined in detail for the sorption thermodynamics and kinetics of hydrogen and also of deuterium, by employing MD combined with Widom averaging towards studying phase equilibria. The latter methodology ensures a rigorous and efficient way for post-processing the dynamics trajectory, thereby avoiding stochastic moves via Monte Carlo simulation, over the large number of configurational degrees of freedom a nonrigid framework encompasses. PMID:23343292
NASA Astrophysics Data System (ADS)
Foglia, Fabrizia; Hazael, Rachael; Simeoni, Giovanna G.; Appavou, Marie-Sousai; Moulin, Martine; Haertlein, Michael; Trevor Forsyth, V.; Seydel, Tilo; Daniel, Isabelle; Meersman, Filip; McMillan, Paul F.
2016-01-01
Quasielastic neutron scattering (QENS) is an ideal technique for studying water transport and relaxation dynamics at pico- to nanosecond timescales and at length scales relevant to cellular dimensions. Studies of high pressure dynamic effects in live organisms are needed to understand Earth’s deep biosphere and biotechnology applications. Here we applied QENS to study water transport in Shewanella oneidensis at ambient (0.1 MPa) and high (200 MPa) pressure using H/D isotopic contrast experiments for normal and perdeuterated bacteria and buffer solutions to distinguish intracellular and transmembrane processes. The results indicate that intracellular water dynamics are comparable with bulk diffusion rates in aqueous fluids at ambient conditions but a significant reduction occurs in high pressure mobility. We interpret this as due to enhanced interactions with macromolecules in the nanoconfined environment. Overall diffusion rates across the cell envelope also occur at similar rates but unexpected narrowing of the QENS signal appears between momentum transfer values Q = 0.7-1.1 Å-1 corresponding to real space dimensions of 6-9 Å. The relaxation time increase can be explained by correlated dynamics of molecules passing through Aquaporin water transport complexes located within the inner or outer membrane structures.
Foglia, Fabrizia; Hazael, Rachael; Simeoni, Giovanna G.; Appavou, Marie-Sousai; Moulin, Martine; Haertlein, Michael; Trevor Forsyth, V.; Seydel, Tilo; Daniel, Isabelle; Meersman, Filip; McMillan, Paul F.
2016-01-01
Quasielastic neutron scattering (QENS) is an ideal technique for studying water transport and relaxation dynamics at pico- to nanosecond timescales and at length scales relevant to cellular dimensions. Studies of high pressure dynamic effects in live organisms are needed to understand Earth’s deep biosphere and biotechnology applications. Here we applied QENS to study water transport in Shewanella oneidensis at ambient (0.1 MPa) and high (200 MPa) pressure using H/D isotopic contrast experiments for normal and perdeuterated bacteria and buffer solutions to distinguish intracellular and transmembrane processes. The results indicate that intracellular water dynamics are comparable with bulk diffusion rates in aqueous fluids at ambient conditions but a significant reduction occurs in high pressure mobility. We interpret this as due to enhanced interactions with macromolecules in the nanoconfined environment. Overall diffusion rates across the cell envelope also occur at similar rates but unexpected narrowing of the QENS signal appears between momentum transfer values Q = 0.7–1.1 Å−1 corresponding to real space dimensions of 6–9 Å. The relaxation time increase can be explained by correlated dynamics of molecules passing through Aquaporin water transport complexes located within the inner or outer membrane structures. PMID:26738409
Foglia, Fabrizia; Hazael, Rachael; Simeoni, Giovanna G; Appavou, Marie-Sousai; Moulin, Martine; Haertlein, Michael; Trevor Forsyth, V; Seydel, Tilo; Daniel, Isabelle; Meersman, Filip; McMillan, Paul F
2016-01-01
Quasielastic neutron scattering (QENS) is an ideal technique for studying water transport and relaxation dynamics at pico- to nanosecond timescales and at length scales relevant to cellular dimensions. Studies of high pressure dynamic effects in live organisms are needed to understand Earth's deep biosphere and biotechnology applications. Here we applied QENS to study water transport in Shewanella oneidensis at ambient (0.1 MPa) and high (200 MPa) pressure using H/D isotopic contrast experiments for normal and perdeuterated bacteria and buffer solutions to distinguish intracellular and transmembrane processes. The results indicate that intracellular water dynamics are comparable with bulk diffusion rates in aqueous fluids at ambient conditions but a significant reduction occurs in high pressure mobility. We interpret this as due to enhanced interactions with macromolecules in the nanoconfined environment. Overall diffusion rates across the cell envelope also occur at similar rates but unexpected narrowing of the QENS signal appears between momentum transfer values Q = 0.7-1.1 Å(-1) corresponding to real space dimensions of 6-9 Å. The relaxation time increase can be explained by correlated dynamics of molecules passing through Aquaporin water transport complexes located within the inner or outer membrane structures. PMID:26738409
Coherent Dynamics of meta-Toluidine Investigated by QuasiElastic Neutron Scattering
Faraone, Antonio; Hong, Kunlun; Kneller, Larry; Ohl, Michael E; Copley, John R. D.
2012-01-01
The coherent dynamics of a typical fragile glass former, meta-toluidine, was investigated at the molecular level using quasielastic neutron scattering, with time-of-flight and neutron spin echo spectrometers. It is well known that the static structure factor of meta-toluidine shows a prepeak originating from clustering of the molecules through hydrogen bonding between the amine groups. The dynamics of meta-toluidine was measured for several values of the wavevector transfer Q, which is equivalent to an inverse length scale, in a range encompassing the prepeak and the structure factor peak. Data were collected in the temperature range corresponding to the liquid and supercooled states, down to the glass transition. At least two dynamical processes were identified. This paper focuses on the slowest relaxation process in the system, the {alpha}-relaxation, which was found to scale with the macroscopic shear viscosity at all the investigated Q values. No evidence of 'de Gennes' narrowing associated with the prepeak was observed, in contrast with what happens at the Q value corresponding to the interparticle distance. Moreover, using partially deuterated samples, the dynamics of the clusters was found to be correlated to the single-particle dynamics of the meta-toluidine molecules.
Kyriakos, Konstantinos; Philipp, Martine; Silvi, Luca; Lohstroh, Wiebke; Petry, Winfried; Müller-Buschbaum, Peter; Papadakis, Christine M
2016-05-26
The solvent dynamics of concentrated solutions of poly(N-isopropylacrylamide) (PNIPAM, 25 wt %) in water/methanol mixtures (85:15 v/v) are measured with the aim of shedding light onto the cononsolvency effect. Quasi-elastic neutron scattering (QENS) with contrast variation has been carried out at temperatures below and above the cloud point by using in the first set of experiments the mixture H2O:d-MeOD (d-MeOD denotes fully deuterated methanol) as a solvent and in the second set of experiments the mixture D2O:MeOH (MeOH denotes methanol). As a reference, bulk H2O, bulk MeOH and the mixtures H2O:d-MeOD and D2O:MeOH (both 85:15 v/v) have been investigated as well. In the PNIPAM solution in H2O:d-MeOD, two water populations are identified, namely strongly and less strongly arrested water. At the cloud point, the former is partially released from PNIPAM. The diffusion coefficient of the latter one is similar to the one in the water/methanol mixture, and its residence time decreases at the cloud point. The PNIPAM solution in D2O:MeOH reveals similar dynamics to the one in H2O:d-MeOD which may reflect that the dynamics of MeOH near the PNIPAM chain is similar to the one of H2O. The similarity may, however, partially be due to H/D exchange between D2O and MeOH. In both PNIPAM solutions, the mean-square displacement of the PNIPAM chain decreases gradually above the cloud point. PMID:27187897
Measurement of the nu(mu) Charged Current pi+ Production to Quasi-elastic Scattering Cross Section
Nowak, Jaroslaw A.; /Louisiana State U.
2009-09-01
Using high statistics samples of charged current interactions, MiniBooNE reports a model independent measurement of the single charged pion production to quasi-elastic cross section ratio on mineral oil without corrections for pion re-interactions in the target nucleus [1]. The result is provided as a function of neutrino energy in the range 0.4 GeV < E < 2.4 GeV with 11% precision in the region of highest statistics.
Breakup coupling effects on near-barrier quasi-elastic scattering of {sup 6,7}Li on {sup 144}Sm
Otomar, D. R.; Lubian, J.; Gomes, P. R. S.; Monteiro, D. S.; Niello, J. O. Fernandez; Guimaraes, V.; Chamon, L. C.
2009-09-15
Excitation functions of quasi-elastic scattering at backward angles have been measured for the {sup 6,7}Li+{sup 144}Sm systems at near-barrier energies, and fusion barrier distributions have been extracted from the first derivatives of the experimental cross sections with respect to the bombarding energies. The data have been analyzed in the framework of continuum discretized coupled-channel calculations, and the results have been obtained in terms of the influence exerted by the inclusion of different reaction channels, with emphasis on the role played by the projectile breakup.
Measurement of quasi-elastic back-scattering of {sup 64}Ni+{sup 118}Sn and {sup 58}Ni+{sup 124}Sn
Watanabe, Y. X.; Jeong, S. C.; Hirayama, Y.; Imai, N.; Ishiyama, H.; Miyatake, H.; Mitsuoka, S.; Nishio, K.; Hashimoto, T.; Ikezoe, H.
2009-05-04
Two systems of {sup 64}Ni+{sup 118}Sn and {sup 58}Ni+{sup 124}Sn produce the same compound nucleus {sup 182}Pt in the fusion reaction and they show the similar fusion cross sections below and near the Coulomb barriers, although only the system of {sup 58}Ni+{sup 124}Sn has positive Q-value multi-neutron transfer channels of 1-11 neutron(s). In order to investigate the possible effect of positive Q-value multi-neutron transfer channels on the capture cross sections, the quasi-elastic back-scattering for the two systems were measured below and near the Coulomb barriers at the backward angles of 162 deg. and 172 deg. The beam energies were altered in the energy range and the quasi-elastic back-scattering excitation functions were obtained. They were compared with the coupled-channel calculations of collective excitations and a two-neutron transfer channel, indicating no evidence of a significant effect of the positive Q-value multi-neutron transfer channels on the capture cross sections for the system of {sup 58}Ni+{sup 124}Sn.
Al-Wahish, Amal; Armitage, D.; Hill, B.; Mills, R.; Santodonato, L.; Herwig, K. W.; Al-Binni, U.; Jalarvo, N.; Mandrus, D.
2015-09-15
A design for a sample cell system suitable for high temperature Quasi-Elastic Neutron Scattering (QENS) experiments is presented. The apparatus was developed at the Spallation Neutron Source in Oak Ridge National Lab where it is currently in use. The design provides a special sample cell environment under controlled humid or dry gas flow over a wide range of temperature up to 950 °C. Using such a cell, chemical, dynamical, and physical changes can be studied in situ under various operating conditions. While the cell combined with portable automated gas environment system is especially useful for in situ studies of microscopic dynamics under operational conditions that are similar to those of solid oxide fuel cells, it can additionally be used to study a wide variety of materials, such as high temperature proton conductors. The cell can also be used in many different neutron experiments when a suitable sample holder material is selected. The sample cell system has recently been used to reveal fast dynamic processes in quasi-elastic neutron scattering experiments, which standard probes (such as electrochemical impedance spectroscopy) could not detect. In this work, we outline the design of the sample cell system and present results demonstrating its abilities in high temperature QENS experiments.
NASA Astrophysics Data System (ADS)
al-Wahish, Amal; Armitage, D.; al-Binni, U.; Hill, B.; Mills, R.; Jalarvo, N.; Santodonato, L.; Herwig, K. W.; Mandrus, D.
2015-09-01
A design for a sample cell system suitable for high temperature Quasi-Elastic Neutron Scattering (QENS) experiments is presented. The apparatus was developed at the Spallation Neutron Source in Oak Ridge National Lab where it is currently in use. The design provides a special sample cell environment under controlled humid or dry gas flow over a wide range of temperature up to 950 °C. Using such a cell, chemical, dynamical, and physical changes can be studied in situ under various operating conditions. While the cell combined with portable automated gas environment system is especially useful for in situ studies of microscopic dynamics under operational conditions that are similar to those of solid oxide fuel cells, it can additionally be used to study a wide variety of materials, such as high temperature proton conductors. The cell can also be used in many different neutron experiments when a suitable sample holder material is selected. The sample cell system has recently been used to reveal fast dynamic processes in quasi-elastic neutron scattering experiments, which standard probes (such as electrochemical impedance spectroscopy) could not detect. In this work, we outline the design of the sample cell system and present results demonstrating its abilities in high temperature QENS experiments.
al-Wahish, Amal; Armitage, D; al-Binni, U; Hill, B; Mills, R; Jalarvo, N; Santodonato, L; Herwig, K W; Mandrus, D
2015-09-01
A design for a sample cell system suitable for high temperature Quasi-Elastic Neutron Scattering (QENS) experiments is presented. The apparatus was developed at the Spallation Neutron Source in Oak Ridge National Lab where it is currently in use. The design provides a special sample cell environment under controlled humid or dry gas flow over a wide range of temperature up to 950 °C. Using such a cell, chemical, dynamical, and physical changes can be studied in situ under various operating conditions. While the cell combined with portable automated gas environment system is especially useful for in situ studies of microscopic dynamics under operational conditions that are similar to those of solid oxide fuel cells, it can additionally be used to study a wide variety of materials, such as high temperature proton conductors. The cell can also be used in many different neutron experiments when a suitable sample holder material is selected. The sample cell system has recently been used to reveal fast dynamic processes in quasi-elastic neutron scattering experiments, which standard probes (such as electrochemical impedance spectroscopy) could not detect. In this work, we outline the design of the sample cell system and present results demonstrating its abilities in high temperature QENS experiments. PMID:26429475
Djurado, David; Bée, Marc; Sniechowski, Maciej; Howells, Spencer; Rannou, Patrice; Pron, Adam; Travers, J P; Luzny, Wojciech
2005-03-21
Proton dynamics in films of poly(aniline) "plastdoped" with di-esters of sulfophthalic (or sulfosuccinic) acids have been investigated by using quasi-elastic neutron scattering techniques. A broad time range (10(-13)-10(-9) s) has been explored by using four different spectrometers. In this time range, the dynamics is exclusively due to protons attached to the flexible tails of the counter-ions. A model of limited diffusion in spheres whose radii are distributed in size gives a realistic view of the geometry of molecular motions. However, it is found that the characteristic times of these motions are widely distributed over several orders of magnitude. The time decay of the intermediate scattering function is well described by a time power law. This behaviour is qualitatively discussed in connection with the structure of the systems and by comparison with other so-called complex systems. PMID:19791338
Guilbert, Anne A Y; Zbiri, Mohamed; Jenart, Maud V C; Nielsen, Christian B; Nelson, Jenny
2016-06-16
The molecular dynamics of organic semiconductor blend layers are likely to affect the optoelectronic properties and the performance of devices such as solar cells. We study the dynamics (5-50 ps) of the poly(3-hexylthiophene) (P3HT): phenyl-C61-butyric acid methyl ester (PCBM) blend by time-of-flight quasi-elastic neutron scattering, at temperatures in the range 250-360 K, thus spanning the glass transition temperature region of the polymer and the operation temperature of an OPV device. The behavior of the QENS signal provides evidence for the vitrification of P3HT upon blending, especially above the glass transition temperature, and the plasticization of PCBM by P3HT, both dynamics occurring on the picosecond time scale. PMID:27192930
NASA Astrophysics Data System (ADS)
Cheoun, Myung-Ki; Kim, K. S.; Kim, Hungchong; So, W. Y.; Maruyama, Tomoyuki; Kajino, Toshitaka
2015-04-01
We investigated the in-medium effect by density-dependent axial and weak-vector form factors on muon-neutrino ({{ν }μ }) and anti-muon-neutrino ({{\\bar{ν }}μ }) scattering in the quasi-elastic (QE) region from nucleons (N*) bound in a nucleus or immersed in a nuclear medium via neutral current (NC) and charged current (CC). For the density-dependent form factors, we exploited a quark-meson-coupling (QMC) model. We found that the {{ν }μ }({{\\bar{ν }}μ })-{{N}*} scattering cross sections via NC in the QE region usually decrease with an increased medium density, while those using CC were increased. However, their rate of change was sensitive to the four-momentum transfer given to a bound nucleon through scattering. We compared these results obtained by the elementary process corrected by the in-medium effect to the BNL and MiniBooNE data, which measured {{ν }μ } scattering cross sections per nucleon through {{ν }μ } - 12C scattering in 12C composite targets. The incident energy range was 550 \\lt {{E}ν }\\lt 3000 MeV. We increased the energy up to 100 GeV to compare our results to the NOMAD experimental data. In order to study the density effects on a nucleon embedded in 12C, we exploited the QMC form factors evaluated at ρ =0.5{{ρ }o}, where the normal density {{ρ }o}˜ 0.15 f{{m}-3}. The strangeness contributions in NC scattering are also incorporated into the form factors for comparison with experimental data. Our numerical results show that most of the experimental data can be explained in a satisfactory manner by the density-dependent elementary process, but there are some remaining deviations resulting from the nuclear structure, particularly in the low and high momentum-transfer regions.
Salles, Fabrice; Jobic, Hervé; Devic, Thomas; Llewellyn, Philip L; Serre, Christian; Férey, Gérard; Maurin, Guillaume
2010-01-26
Quasi-elastic neutron scattering measurements are combined with molecular dynamics simulations to determine the self-diffusivity, corrected diffusivity, and transport diffusivity of CO(2) in the metal-organic framework MIL-47(V) (MIL = Materials Institut Lavoisier) over a wide range of loading. The force field used for describing the host/guest interactions is first validated on the thermodynamics of the MIL-47(V)/CO(2) system, prior to being transferred to the investigations of the dynamics. A decreasing profile is then deduced for D(s) and D(o) whereas D(t) presents a non monotonous evolution with a slight decrease at low loading followed by a sharp increase at higher loading. Such decrease of D(t) which has never been evidenced in any microporous systems comes from the atypical evolution of the thermodynamic correction factor that reaches values below 1 at low loading. This implies that, due to intermolecular interactions, the CO(2) molecules in MIL-47(V) do not behave like an ideal gas. Further, molecular simulations enabled us to elucidate unambiguously a 3D diffusion mechanism within the pores of MIL-47(V). PMID:19957953
Mavila Chathoth, Suresh; Mamontov, Eugene; Melnichenko, Yuri B; Zamponi, Michaela M
2010-01-01
The diffusion of methane confined in nano-porous carbon aerogel with the average pore size 48 {angstrom} and porosity 60% was investigated as a function of pressure at T = 298 K using quasi-elastic neutron scattering (QENS). The diffusivity of methane shows a clear effect of confinement: it is about two orders of magnitude lower than in bulk at the same thermodynamic conditions and is close to the diffusivity of liquid methane at 100 K (i.e. {approx} 90 K below the liquid-gas critical temperature T{sub C} {approx} 191 K). The diffusion coefficient (D) of methane initially increases with pressure by a factor of {approx}2.5 from 3.47 {+-} 0.41 x 10{sup -10} m{sup 2} s{sup -1} at 0.482 MPa to D = 8.55 {+-} 0.33 x 10{sup -10} m{sup 2} s{sup -1} at 2.75 MPa and starts to decrease at higher pressures. An explanation of the observed non-monotonic behavior of the diffusivity in the confined fluid is based on the results of small-angle neutron scattering experiments of the phase behavior of methane in a similar carbon aerogel sample. The initial increase of the diffusion coefficient with pressure is explained as due to progressive filling of bigger pores in which molecular mobility in the internal pore volume is less affected by the sluggish liquid-like molecular mobility in the adsorbed phase. Subsequent decrease of D, is associated with the effect of intermolecular collisions, which result in a lower total molecular mobility with pressure, as in the bulk state. The results are compared with the available QENS data on the methane diffusivity in zeolites, metal organic frameworks, and porous silica as well as with the molecular dynamics simulations of methane in nano-porous carbons and silica zeolites.
Etampawala, Thusitha; Ratnaweera, Dilru; Morgan, Brian; Diallo, Souleymane; Mamontov, Eugene; Dadmun, Mark
2015-02-02
Our work reports on the detailed molecular dynamic behavior of miscible blends of Poly(3-hexylthiophene) (P3HT) and [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) and their pure counterparts by quasi-elastic neutron scattering measurements (QENS). The study provides the measure of relaxation processes on pico-to-nanosecond time scales. A single relaxation process was observed in pure P3HT and PCBM while two relaxation processes, one fast and one slow, were observed in the blends. The fast process was attributed to the dynamics of P3HT while the slow process was correlated to the dynamics of PCBM. The results show that the relaxation process is a balance between two opposing effects: increased mobility due to thermal activation of P3HT molecules and decrease mobility due to the presence of PCBM which is correlated to the percent crystallinity of P3HT and local packing density of PCBM in the amorphous phase. The threshold for the domination of the thermally activated relaxation is between 5 and 9 vol.% of PCBM loading. Two distinct spatial dependences of the relaxation processes, in which the crossover length scale depends neither on temperature nor composition, were observed for all the samples. They were attributed to the collective motions of the hexyl side chains and the rotational motions of the C-C single bonds of the side chains. Finally, these results provide an understanding of the effects of PCBM loading and temperature on the dynamics of the polymer-fullerene blends which provides a tool to optimize the efficiency of charge carrier and exciton transport within the organic photovoltaic (OPV) active layer to improve the high performance of organic solar cells.
Etampawala, Thusitha; Ratnaweera, Dilru; Morgan, Brian; Diallo, Souleymane; Mamontov, Eugene; Dadmun, Mark
2015-02-02
Our work reports on the detailed molecular dynamic behavior of miscible blends of Poly(3-hexylthiophene) (P3HT) and [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) and their pure counterparts by quasi-elastic neutron scattering measurements (QENS). The study provides the measure of relaxation processes on pico-to-nanosecond time scales. A single relaxation process was observed in pure P3HT and PCBM while two relaxation processes, one fast and one slow, were observed in the blends. The fast process was attributed to the dynamics of P3HT while the slow process was correlated to the dynamics of PCBM. The results show that the relaxation process is a balance betweenmore » two opposing effects: increased mobility due to thermal activation of P3HT molecules and decrease mobility due to the presence of PCBM which is correlated to the percent crystallinity of P3HT and local packing density of PCBM in the amorphous phase. The threshold for the domination of the thermally activated relaxation is between 5 and 9 vol.% of PCBM loading. Two distinct spatial dependences of the relaxation processes, in which the crossover length scale depends neither on temperature nor composition, were observed for all the samples. They were attributed to the collective motions of the hexyl side chains and the rotational motions of the C-C single bonds of the side chains. Finally, these results provide an understanding of the effects of PCBM loading and temperature on the dynamics of the polymer-fullerene blends which provides a tool to optimize the efficiency of charge carrier and exciton transport within the organic photovoltaic (OPV) active layer to improve the high performance of organic solar cells.« less
NASA Astrophysics Data System (ADS)
Wolcott, Jeremy
We report herein the first-ever measurement of a cross-section for an exclusive state in electron neutrino scattering at the GeV scale, which was made using the MINERnuA detector in the NuMI neutrino beam at Fermilab. We present the electron neutrino CCQE differential cross-sections, which are averaged over neutrinos of energies 1-10 GeV (with mean energy of about 3 GeV), in terms of various kinematic variables: final-state electron angle, final-state electron energy, and the square of the four-momentum transferred to the nucleus by the neutrino, Q2. We also provide a total cross-section vs. neutrino energy. While our measurement of this process is found to be in agreement with the predictions of the GENIE event generator, we also report on an unpredicted photon-like process we observe in a similar kinematic regime. The absence of this process from models for neutrino interactions is a potential stumbling block for future on-axis neutrino oscillation experiments. We include kinematic and particle species identification characterizations which can be used in building models to help address this shortcoming.
Wang Xu; Dipangkar Dutta; Feng Xiong; Brian Anderson; Leonard Auerbach; Todd Averett; William Bertozzi; Tim Black; John Calarco; Lawrence Cardman; Gordon Cates; Zhengwei Chai; Jian-ping Chen; Seonho Choi; Eugene Chudakov; Steve Churchwell; G.S. Corrado; C. Crawford; Daniel Dale; Alexandre Deur; Pibero Djawotho; Bradley Filippone; John Finn; Haiyan Gao; Ronald Gilman; Oleksandr Glamazdin; Charles Glashausser; Walter Gloeckle; J. Golak; Javier Gomez; Viktor Gorbenko; Jens-ole Hansen; F. Hersman; Douglas Higinbotham; Richard Holmes; Calvin Howell; Emlyn Hughes; Thomas Humensky; Sebastien Incerti; Cornelis De Jager; John Jensen; Xiaodong Jiang; C.E. Jones; Mark Jones; R. Kahl; H. Kamada; A. Kievsky; Ioannis Kominis; Wolfgang Korsch; Kevin Kramer; Gerfried Kumbartzki; Michael Kuss; Enkeleida Lakuriqi; Meihua Liang; Nilanga Liyanage; John Lerose; Sergey Malov; Demetrius Margaziotis; J.W. Martin; Kathy Mccormick; Robert Mckeown; Kevin Mcilhany; Zein-eddine Meziani; Robert Michaels; G.W. Miller; Joseph Mitchell; Sirish Nanda; E. Pace; Tina Pavlin; Gerassimos Petratos; Roman Pomatsalyuk; D. Pripstein; David Prout; Ronald Ransome; Yves Roblin; Marat Rvachev; Arunava Saha; G. Salme; Michael Schnee; Taeksu Shin; Karl Slifer; Paul Souder; Steffen Strauch; Riad Suleiman; Mark Sutter; Bryan Tipton; Luminita Todor; Michele Viviani; Branislav Vlahovic; J. Watson; Claude Williamson; H. Witala; Bogdan Wojtsekhowski; Jen-chuan Yeh; Piotr Zolnierczuk
2000-10-01
We have measured the transverse asymmetry from inclusive scattering of longitudinally polarized electrons from polarized {sup 3}He nuclei at quasi-elastic kinematics in Hall A at Jefferson Lab with high statistical and systematic precision. The neutron magnetic form factor was extracted based on Faddeev calculations with an experimental uncertainty of less than 2%.
Studying neutrino oscillations using quasi-elastic events in MINOS
Kumaratunga, Sujeewa Terasita; /Minnesota U.
2008-02-01
MINOS (Main Injector Neutrino Oscillation Search), is a long baseline neutrino experiment designed to search for neutrino oscillations using two detectors at Fermi National Accelerator Laboratory, IL (Near Detector) and Soudan, MN (Far Detector). It will study {nu}{sub {mu}} {yields} {nu}{sub {tau}} oscillations and make a measurement on the oscillation parameters, {Delta}m{sub 23}{sup 2} and sin{sup 2} 2{theta}{sub 23}, via a {nu}{sub {mu}} beam made at Fermilab. Charge current neutrino interactions in the MINOS detectors are of three types: quasi-elastic scattering (QEL), resonance scattering (RES) and deep inelastic scattering (DIS). Of these, quasi-elastic scattering leaves the cleanest signal with just one {mu} and one proton in the final state, thus rendering the reconstruction of the neutrino energy more accurate. This thesis will outline a method to separate QEL events from the others in the two detectors and perform a calculation of {Delta}m{sub 23}{sup 2} and sin{sup 2} 2{theta}{sub 23} using those events. The period under consideration was May 2005 to February 2006. The number of observed quasi-elastic events with energies below 10 GeV was 29, where the expected number was 60 {+-} 3. A fit to the energy distribution of these events gives {Delta}m{sub 23}{sup 2} = 2.91{sub -0.53}{sup +0.49}(stat){sub -0.09}{sup +0.08}(sys) x 10{sup -3} eV{sup 2} and sin{sup 2} 2{theta}{sub 23} = 0.990{sub -0.180}(stat){sub -0.030}(sys).
Longitudinal and Transverse Quasi-Elastic Response Functions of Light Nuclei
J. Carlson; J. Jourdan; R. Schiavilla; I. Sick
2001-06-01
The {sup 3}He and {sup 4}He longitudinal and transverse response functions are determined from an analysis of the world data on quasi-elastic inclusive electron scattering. The corresponding Euclidean response functions are derived and compared to those calculated with Green's function Monte Carlo methods, using realistic interactions and currents. Large contributions associated with two-body currents are found, particularly in the {sup 4}He transverse response, in agreement with data. The contributions of two-body charge and current operators in the {sup 3}He, {sup 4}He, and {sup 6}Li response functions are also studied via sum-rule techniques. A semi-quantitative explanation for the observed systematics in the excess of transverse quasi-elastic strength, as function of mass number and momentum transfer, is provided. Finally, a number of model studies with simplified interactions, currents, and wave functions is carried out to elucidate the role played, in the full calculation, by tensor interactions and correlations.
Inclusive Inelastic Electron Scattering from Nuclei
Fomin, Nadia
2007-10-26
Inclusive electron scattering from nuclei at large x and Q{sup 2} is the result of a reaction mechanism that includes both quasi-elastic scattering from nucleons and deep inelastic scattering from the quark consitituents of the nucleons. Data in this regime can be used to study a wide variety of topics, including the extraction of nuclear momentum distributions, the infiuence of final state interactions and the approach to y-scaling, the strength of nucleon-nucleon correlations, and the approach to x-scaling, to name a few. Selected results from the recent experiment E02-019 at the Thomas Jefferson National Accelerator Facility will be shown and their relevance discussed.
Deriving capture and reaction cross sections from observed quasi-elastic and elastic backscattering
NASA Astrophysics Data System (ADS)
Sargsyan, V. V.; Adamian, G. G.; Antonenko, N. V.; Diaz-Torres, A.; Gomes, P. R. S.; Lenske, H.
2014-12-01
Based on reaction theory, we suggest a useful method for extracting total and partial reaction and capture (complete fusion) cross sections from the experimental elastic and quasi-elastic backscattering excitation functions taken at a single angle. We also propose a method to predict the differential reaction cross section from the observed elastic-scattering angular distribution.
How well do we understand quasi-elastic reactions at energies close to the barrier
Rehm, K.E.
1988-01-01
In collisions between too heavy nuclei a wide spectrum of different reaction modes is observed covering the range from simple processes like elastic scattering to complicated multistep transfers and fusion. On the theoretical side heavy ion reactions are usually analyzed using models that were developed first for light ion induced reactions: the optical model for elastic scattering and the DWBA for more inelastic processes like transfer and inelastic scattering. Some of the assumptions going into these approximations, however, are not valid for heavy ion induced reactions. The region between fusion and quasi-elastic reactions is not well understood theoretically. This region is associated with deep inelastic collisions, which are complex multiparticle reactions involving transfer of several protons and neutrons. In this paper, the author discusses to what extent experiments in the field of quasi-elastic scattering are understood within the framework of various theoretical models and in what areas more work is needed.
Charged current quasi-elastic neutrino analysis at MINERνA
Fiorentini, G. A.
2015-05-15
MINERνA (Main INjector Experiment for ν-A) is a neutrino scattering experiment in the NuMI high-intensity neutrino beam at the Fermi National Accelerator Laboratory. MINERvA was designed to make precision measurements of low energy neutrino and antineutrino cross sections on a variety of different materials (plastic scintillator, C, Fe, Pb, He and H2O). We present the current status of the charged current quasi-elastic scattering in plastic scintillator.
Effective Spectral Function for Neutrino Quasielastic Scattering Event Generators
NASA Astrophysics Data System (ADS)
Coopersmith, Brian; Bodek, Arie; Christy, M. Eric
2014-03-01
The spectral functions that are used in modeling of quasi elastic scattering in neutrino event generators such as GENIE, NEUT, NUANCE and NUWRO event generators include (Global) Fermi gas, local Fermi gas, Bodek-Ritche Fermi gas with high momentum tail, and the Benhar Fantoni spectral function. We find that these spectral functions do not agree with the prediction of ψ' superscaling functions that are extracted from electron quasi elastic scattering data on nuclear targets. It is known that spectral functions do not fully describe quasi elastic scattering because they only model the initial state. Final state interactions distort the shape of the quasi elastic peak, reduce the cross section at the peak and increase the cross section at the tail of the distribution for large energy transfer to final state nucleons. We show that an ``effective spectral function'' can be constructed to reliably reproduce the kinematic distributions predicted by the ψ' super scaling formalism.
Experimental elastic and quasi-elastic angular distributions provide transfer probabilities
NASA Astrophysics Data System (ADS)
Sargsyan, V. V.; Adamian, G. G.; Antonenko, N. V.; Diaz-Torres, A.; Gomes, P. R. S.; Lenske, H.
2016-05-01
Following a similar approach suggested recently to derive breakup probabilities [Phys. Rev. C 92, 054620 (2015), 10.1103/PhysRevC.92.054620], we present a simple method to derive transfer probabilities by measuring only elastic or quasi-elastic scattering for the system under investigation with the positive transfer Q values and a similar system with closed transfer channels. Our estimations and transfer data for the two-neutron stripping in the 18O+206Pb reaction are in a reasonable agreement.
Electron scattering from pyrimidine
NASA Astrophysics Data System (ADS)
Colmenares, Rafael; Fuss, Martina C.; Oller, Juan C.; Muñoz, Antonio; Blanco, Francisco; Almeida, Diogo; Limão-Vieira, Paulo; García, Gustavo
2014-04-01
Electron scattering from pyrimidine (C4H4N2) was investigated over a wide range of energies. Following different experimental and theoretical approaches, total, elastic and ionization cross sections as well as electron energy loss distributions were obtained.
Nanowire electron scattering spectroscopy
NASA Technical Reports Server (NTRS)
Hunt, Brian D. (Inventor); Bronikowski, Michael (Inventor); Wong, Eric W. (Inventor); von Allmen, Paul (Inventor); Oyafuso, Fabiano A. (Inventor)
2009-01-01
Methods and devices for spectroscopic identification of molecules using nanoscale wires are disclosed. According to one of the methods, nanoscale wires are provided, electrons are injected into the nanoscale wire; and inelastic electron scattering is measured via excitation of low-lying vibrational energy levels of molecules bound to the nanoscale wire.
Transition from quasi-elastic to deep-inelastic reactions
Rehm, K.E.
1986-01-01
Heavy ion induced transfer reactions are usually considered to fall into two categories. Quasi-elastic processes, on one hand, are characterized by small energy transfers, with one-nucleon transfer reactions being a typical example. These processes are dominant for grazing collisions, and are generally described within simple one-step DWBA calculations. Deep inelastic reactions, on the other hand, occur for more central collisions where the interaction time is longer and subsequently more energy and particles can be exchanged. Quasi-elastic collisions dominate transfer reactions induced by light heavy ions (e.g., /sup 16/O) at energies not too high above the barrier, while deep inelastic collisions are observed mainly in reactions induced by heavier projectiles (Kr, Xe). In this contribution, we discuss the transition between these two processes for the system /sup 48/Ti + /sup 208/Pb. /sup 48/Ti is located between light (/sup 16/O) and heavy (Kr) projectiles and should be well suited for a study of the interrelation between quasi- and deep-inelastic reactions. The experiments were performed with a 300 MeV /sup 48/Ti beam obtained from the Argonne National Laboratory superconducting linac. The outgoing particles were momentum analyzed in a split pole magnetic spectrograph and detected in the focal plane by a position sensitive ionization chamber. The specific energy loss, the magnetic rigidity and the total energy of the outgoing particles were measured enabling mass and Z-identification. The energy resolution was about 3 MeV, determined by the thickness of the /sup 208/Pb target, and thus excluded study of transfer reactions to discrete final states. Angular distributions were measured in the range theta/sub lab/ = 20/sup 0/ to 80/sup 0/ in steps of 5/sup 0/. 8 refs.
Nanowire Electron Scattering Spectroscopy
NASA Technical Reports Server (NTRS)
Hunt, Brian; Bronikowsky, Michael; Wong, Eric; VonAllmen, Paul; Oyafuso, Fablano
2009-01-01
Nanowire electron scattering spectroscopy (NESS) has been proposed as the basis of a class of ultra-small, ultralow-power sensors that could be used to detect and identify chemical compounds present in extremely small quantities. State-of-the-art nanowire chemical sensors have already been demonstrated to be capable of detecting a variety of compounds in femtomolar quantities. However, to date, chemically specific sensing of molecules using these sensors has required the use of chemically functionalized nanowires with receptors tailored to individual molecules of interest. While potentially effective, this functionalization requires labor-intensive treatment of many nanowires to sense a broad spectrum of molecules. In contrast, NESS would eliminate the need for chemical functionalization of nanowires and would enable the use of the same sensor to detect and identify multiple compounds. NESS is analogous to Raman spectroscopy, the main difference being that in NESS, one would utilize inelastic scattering of electrons instead of photons to determine molecular vibrational energy levels. More specifically, in NESS, one would exploit inelastic scattering of electrons by low-lying vibrational quantum states of molecules attached to a nanowire or nanotube.
NASA Astrophysics Data System (ADS)
Androić, D.; Armstrong, D. S.; Arvieux, J.; Asaturyan, R.; Averett, T. D.; Bailey, S. L.; Batigne, G.; Beck, D. H.; Beise, E. J.; Benesch, J.; Benmokhtar, F.; Bimbot, L.; Birchall, J.; Biselli, A.; Bosted, P.; Breuer, H.; Brindza, P.; Capuano, C. L.; Carlini, R. D.; Carr, R.; Chant, N.; Chao, Y.-C.; Clark, R.; Coppens, A.; Covrig, S. D.; Cowley, A.; Dale, D.; Davis, C. A.; Ellis, C.; Falk, W. R.; Fenker, H.; Finn, J. M.; Forest, T.; Franklin, G.; Frascaria, R.; Furget, C.; Gaskell, D.; Gericke, M. T. W.; Grames, J.; Griffioen, K. A.; Grimm, K.; Guillard, G.; Guillon, B.; Guler, H.; Gustafsson, K.; Hannelius, L.; Hansknecht, J.; Hasty, R. D.; Hawthorne Allen, A. M.; Horn, T.; Ito, T. M.; Johnston, K.; Jones, M.; Kammel, P.; Kazimi, R.; King, P. M.; Kolarkar, A.; Korkmaz, E.; Korsch, W.; Kox, S.; Kuhn, J.; Lachniet, J.; Laszewski, R.; Lee, L.; Lenoble, J.; Liatard, E.; Liu, J.; Lung, A.; MacLachlan, G. A.; Mammei, J.; Marchand, D.; Martin, J. W.; Mack, D. J.; McFarlane, K. W.; McKee, D. W.; McKeown, R. D.; Merchez, F.; Mihovilovic, M.; Micherdzinska, A.; Mkrtchyan, H.; Moffit, B.; Morlet, M.; Muether, M.; Musson, J.; Nakahara, K.; Neveling, R.; Niccolai, S.; Nilsson, D.; Ong, S.; Page, S. A.; Papavassiliou, V.; Pate, S. F.; Phillips, S. K.; Pillot, P.; Pitt, M. L.; Poelker, M.; Porcelli, T. A.; Quéméner, G.; Quinn, B. P.; Ramsay, W. D.; Rauf, A. W.; Real, J.-S.; Ries, T.; Roche, J.; Roos, P.; Rutledge, G. A.; Schaub, J.; Secrest, J.; Seva, T.; Simicevic, N.; Smith, G. R.; Spayde, D. T.; Stepanyan, S.; Stutzman, M.; Suleiman, R.; Tadevosyan, V.; Tieulent, R.; van de Wiele, J.; van Oers, W. T. H.; Versteegen, M.; Voutier, E.; Vulcan, W. F.; Wells, S. P.; Warren, G.; Williamson, S. E.; Woo, R. J.; Wood, S. A.; Yan, C.; Yun, J.; Zeps, V.
2011-08-01
In the G0 experiment, performed at Jefferson Lab, the parity-violating elastic scattering of electrons from protons and quasi-elastic scattering from deuterons is measured in order to determine the neutral weak currents of the nucleon. Asymmetries as small as 1 part-per-million in the scattering of a polarized electron beam are determined using a dedicated apparatus. It consists of specialized beam monitoring and control systems, a cryogenic hydrogen (or deuterium) target, and a superconducting, toroidal magnetic spectrometer equipped with plastic scintillation and aerogel Cherenkov detectors, as well as fast readout electronics for the measurement of individual events. The overall design and performance of this experimental system is discussed.
Derivation of capture cross sections from quasi-elastic excitation functions
NASA Astrophysics Data System (ADS)
Sargsyan, V. V.; Adamian, G. G.; Antonenko, N. V.; Gomes, P. R. S.
2013-04-01
The relationship between the quasi-elastic excitation function and the capture cross section is derived. The quasi-elastic data is shown to be a useful tool to extract the capture cross sections and the angular momenta of the captured systems for the reactions 16O+144,154Sm,208Pb, 20Ne+208Pb, and 32S+90,96Zr near and above the Coulomb barrier energies.
A sub-GeV charged-current quasi-elastic $\
Walding, Joseph James
2009-12-01
Neutrino-nucleus charged-current quasi-elastic scattering is the signal interaction used by many neutrino oscillation experiments. For muon disappearance studies the signal mode is ν_{μ}n → μp. Modern oscillation experiments, such as T2K, produce neutrino beams with peak beam energies of order a few-GeV. It is therefore vitally important to have accurate measurements of the charged-current quasi-elastic crosssection for future neutrino oscillation experiments. Neutrino-nucleus cross-sections in the few-GeV region are not well understood, with the main uncertainties coming from understanding of the neutrino beam flux and the final state interactions within nuclei. SciBooNE is a sub-GeV neutrino-nucleus cross-section experiment based at Fermilab, Batavia, USA, with the goal to measure neutrino cross-sections with precision of order 5%. SciBooNE took data from June 2007 until August 2008, in total 0.99×10^{20} and 1.53×10^{20} protons on target were collected in neutrino and anti-neutrino mode, respectively. In this thesis a ν_{μ} charged-current quasi-elastic (CCQE) cross-section contained within the SciBar sub-detector is presented. A method to tag muons in SciBar was developed and three samples were isolated. An excess in backwards tracks in the one-track sample is observed. A Poisson maximum likelihood is used to extract the CCQE cross-section. The fit was applied using a basic fit parameter model, successfully used to obtain the cross-section in the SciBar-MRD matched CCQE analysis. This method was found to be insufficient in describing the data for the SciBarcontained CCQE analysis. By adding two migration parameters the cross-section was calculated to be 1.004 ± 0.031 (stat)^{+0.101} _{-0.150}(sys) × 10^{-38} cm^{2}/neutron, excluding backwards tracks with a χ^{2} = 203.8/76 d.o.f. and 1.083 ± 0.030(stat)^{+0.115} _{-0.177}(sys) × 10^{-38} cm^{2 }
Concept of a multichannel spin-resolving electron analyzer based on Mott scattering
Strocov, Vladimir N.; Petrov, Vladimir N.; Dil, J. Hugo
2015-01-01
The concept of a multichannel electron spin detector based on optical imaging principles and Mott scattering (iMott) is presented. A multichannel electron image produced by a standard angle-resolving (photo) electron analyzer or microscope is re-imaged by an electrostatic lens at an accelerating voltage of 40 kV onto the Au target. Quasi-elastic electrons bearing spin asymmetry of the Mott scattering are imaged by magnetic lenses onto position-sensitive electron CCDs whose differential signals yield the multichannel spin asymmetry image. Fundamental advantages of this concept include acceptance of inherently divergent electron sources from the electron analyzer or microscope focal plane as well as small aberrations achieved by virtue of high accelerating voltages, as demonstrated by extensive ray-tracing analysis. The efficiency gain compared with the single-channel Mott detector can be a factor of more than 104 which opens new prospects of spin-resolved spectroscopies in application not only to standard bulk and surface systems (Rashba effect, topological insulators, etc.) but also to buried heterostructures. The simultaneous spin detection combined with fast CCD readout enables efficient use of the iMott detectors at X-ray free-electron laser facilities. PMID:25931087
NASA Astrophysics Data System (ADS)
Sargsyan, V. V.; Adamian, G. G.; Antonenko, N. V.; Gomes, R. P. S.
2014-12-01
Experimental quasi-elastic backscattering and capture (fusion) excitation functions are usually used to extract the s -wave capture probabilities for the heavy-ion reactions. We investigated the 16O + 120Sn , 144Sm , 208Pb systems at energies near and below the corresponding interaction barriers and concluded that the probabilities extracted from quasi-elastic data are much larger than the ones extracted from fusion excitation functions at sub and deep-sub barrier energies. This seems to be a reasonable explanation for the known disagreement observed in the literature for the nuclear potential diffuseness derived from both methods.
Electron Scattering and Nuclear Structure
ERIC Educational Resources Information Center
Trower, W. P.; Ficenec, J. R.
1971-01-01
Presents information about the nucleus gained by studies of electron scattering. Discusses what can be implied about the shape of the charge distribution, the nucleus positions, the vibrational modes of the nucleus, the momentum of the nucleus, and the granularity and core structures of the nucleus. (DS)
Parity Violation in Electron Scattering
Beise, Elizabeth
2007-10-26
About thirty years ago, electron scattering from nucleons was used [1] to identify, and then measure, the properties of the weak interaction, the only force of nature known to violate the symmetry parity. The basic technique has not fundamentally changed, which is to look for a small asymmetry in count rate from scattering a polarized electron beam from an unpolarized target. Since then, parity-violating (PV) electron scattering has developed substantially, a result of significant improvements in polarized electron beams, accelerator advancements, and developments in cryogenic targets that make it possible to carry out experiments with much higher statistical precision. In the last decade PV experiments have focused on using the complementary electron-quark flavor coupling of the weak interaction to identify and place limits on contributions of strange quark-antiquark pairs to the charge and magnetism of the proton. This observable provides a unique window into the structure of the proton since strange quark contributions can arise only from the sea of quarks and gluons that are responsible for the vast majority of the nucleon's mass. This paper will report on recent results aimed at this goal, along with a brief overview of future directions.
Rukhlenko, Ivan D; Fedorov, Anatoly V; Baymuratov, Anvar S; Premaratne, Malin
2011-08-01
We develop a low-temperature theory of quasi-elastic secondary emission from a semiconductor quantum dot, the electronic subsystem of which is resonant with the confined longitudinal-optical (LO) phonon modes. Our theory employs a generalized model for renormalization of the quantum dot's energy spectrum, which is induced by the polar electron-phonon interaction. The model takes into account the degeneration of electronic states and allows for several LO-phonon modes to be involved in the vibrational resonance. We give solutions to three fundamental problems of energy-spectrum renormalization--arising if one, two, or three LO-phonon modes resonantly couple a pair of electronic states--and discuss the most general problem of this kind that admits an analytical solution. With these results, we solve the generalized master equation for the reduced density matrix, in order to derive an expression for the differential cross section of secondary emission from a single quantum dot. The obtained expression is then analyzed to establish the basics of optical spectroscopy for measuring fundamental parameters of the quantum dot's polaron-like states. PMID:21934910
Spectroscopic study of sub-barrier quasi-elastic nuclear reactions
Pass, C.N.; Evans, P.M.; Smith, A.E.; Stuttge, L.; Betts, R.R.; Lilley, J.S.; Connell, K.A.; Simpson, J.; Smith, J.R.; James, A.N.
1988-01-01
The technique developed in this paper is particularly well suited to the detailed spectroscopic study of low energy quasi-elastic nuclear reactions and by overcoming the limitations of conventional procedure, the prospect of detailed studies of inclusive reaction mechanism may be realised. With only limited statistics we find evidence for strong multistep character in the transfer of a single nucleon from spherical vibrational target to spherical projectile nuclei. The suggestive measurements reported here may be made definitive through extended runs based on this technique and experiments planned for the future offer the real prospect of developing a quantified interpretation of the reaction process. 9 refs. 5 figs.
Parity violation in electron scattering
NASA Astrophysics Data System (ADS)
Souder, P.; Paschke, K. D.
2016-02-01
By comparing the cross sections for left- and right-handed electrons scattered from various unpolarized nuclear targets, the small parity-violating asymmetry can be measured. These asymmetry data probe a wide variety of important topics, including searches for new fundamental interactions and important features of nuclear structure that cannot be studied with other probes. A special feature of these experiments is that the results are interpreted with remarkably few theoretical uncertainties, which justifies pushing the experiments to the highest possible precision. To measure the small asymmetries accurately, a number of novel experimental techniques have been developed.
Electron-Hydrogen Elastic Scattering
NASA Technical Reports Server (NTRS)
Bhatia, A. K.
2004-01-01
Scattering by single-electron systems is always of interest because the wave function of the target is known exactly. Various approximations have been employed to take into account distortion produced in the target. Among them are the method of polarized orbitals and the close coupling approximation. Recently, e-H and e-He+ S-wave scattering in the elastic region has been studied using the Feshbach projection operator formalism. In this approach, the usual Hartree-Fock and exchange potentials are augmented by an optical potential and the resulting phase shifts have rigorous lower bounds. Now this method is being applied to the e-H P-wave scattering in the elastic region. The number of terms in the Hylleraas-type wave function for the 1,3 P phase shifts is 84 and the resulting phase shifts (preliminary) are given. The results have been given up to five digits because to that accuracy they are rigorous lower bounds. They are in general agreement with the variational (VAR) results of Armstead, and those obtained from the intermediate energy R-matrix method (RM) of Scholz et al., and the finite element method (FEM) of Botero and Shertzer. The later two methods do not provide any bounds on phase shifts.
Transient ions in electron and positron scattering
NASA Astrophysics Data System (ADS)
d'A Sanchez, Sergio; de Oliveira, Eliane M.; dos Santos, Josué S.; da Costa, Romarly F.; Bettega, Márcio H. F.; Lima, Marco A. P.; Varella, Márcio T. do N.
2009-11-01
We report on recent advances in studies of transient ions formed in electron and positron scattering by molecules. We briefly discuss elastic electron collisions against pyrrole and glycine, as well as electron affinities of glycine-water clusters. Positron scattering and annihilation on small molecules is also discussed.
Wang Xu
2002-06-01
Electromagnetic form factors are fundamental quantities in describing the underlying electromagnetic structure of nucleons. While proton electromagnetic form factors have been determined with good precision, neutron form factors are known poorly, largely due to the lack of free neutron targets. Jefferson Lab Hall A experiment E95-001, a ''precise measurement of the transverse asymmetry A{sub T}' from the quasielastic {sup 3}He(e, e') process,'' was therefore designed to determine precisely the neutron magnetic form factor, G{sub M}{sup n} at low momentum transfer values and was successfully completed in Spring 1999. High precision A{sub T}'data in the quasi-elastic region at Q{sup 2} values of 0.1 to 0.6 (GeV/c){sup 2} were obtained using a high-pressure spin-exchange optically-pumped polarized {sup 3}He gas target with an average polarization of 30%, a longitudinally polarized e{sup -} beam, and two High Resolution Spectrometers: HRSe and HRSh. HRSe was employed to detect scattered electrons from the quasi-elastic kinematic region, and HRSh was employed as a elastic polarimetry to monitor the product of the beam and target polarizations. The extraction of form factors is usually model-dependent. Significant constraints on theoretical calculations are provided bu additional high precision quasi-elastic asymmetry data at Q{sup 2} values of 0.1 and 0.2 (GeV/c){sup 2} in {sup 3}He breakup region, where effects of final state interactions (FSI) and meson exchange currents (MEC) are expected to be large [71]. G{sub M}{sup n} is extracted from a non-relativistic Faddeev calculation which includes both FSI and MEC at Q{sup 2} values of 0.1 and 0.2 (GeV/c){sup 2}. The uncertainties of G{sub M}{sup n} at these Q{sup 2} values are comparable to those of recent experiments with deuterium targets [58]. At the higher Q{sup 2} values from this experiment, G{sub M}{sup n} is extracted from Plane-Wave Impulsive Approximation (PWIA) calculations with a relatively large theoretical
Positronium and Electron Scattering on Helium
NASA Technical Reports Server (NTRS)
DiRienzi, Joseph
2011-01-01
A recent work [1] establishes experimentally that Positronium scattering by atoms of various elements is surprisingly close in total cross-section to that of an isolated electron of the same velocity. In this work we will look at the scattering of Ps on Helium and compare it to a determination of the scattering of an e- with the same element. For both the Ps scattering and the e- scattering on He, we assume the symmetrization of the e- with the closed shell He electrons is the dominant interaction. A local effective potential employed in [2] and [3] is used to model the electron exchange and cross- sections are determined for a set of partial waves. For the Ps scattering we include as a secondary effect the Van der Waals interaction. For single e- scattering of He, we also employ a short range Coulomb potential and dispersion as contributing effects. Results of the cross-sections determined in each case are then compared
Search for neutrino oscillations in the MINOS experiment by using quasi-elastic interactions
Piteira, Rodolphe; /Paris U., VI-VII
2005-09-01
The enthusiasm of the scientific community for studying oscillations of neutrinos is equaled only by the mass of their detectors. The MINOS experiment determines and compares the near spectrum of muonic neutrinos from the NUMI beam to the far one, in order to measure two oscillation parameters: {Delta}m{sub 23}{sup 2} and sin{sup 2} (2{theta}{sub 23}). The spectra are obtained by analyzing the charged current interactions which difficulty lies in identifying the interactions products (e.g. muons). An alternative method identifying the traces of muons, bent by the magnetic field of the detectors, and determining their energies is presented in this manuscript. The sensitivity of the detectors is optimal for the quasi-elastic interactions, for which a selection method is proposed, to study their oscillation. Even though it reduces the statistics, such a study introduces fewer systematic errors, constituting the ideal method on the long range.
Yamada, Takeshi; Yonamine, Ryo; Yamada, Teppei; Kitagawa, Hiroshi; Tyagi, Madhusudan; Nagao, Michihiro; Yamamuro, Osamu
2011-11-24
We have investigated the mechanism of the first order transition and proton conductivity in copper rubeanate hydrates from microscopic and dynamical points of view. Three different types of neutron spectrometer-time-of-flight, backscattering, and neutron spin echo-were used to cover a wide dynamic range (1 ps to 100 ns). We found that the water molecules adsorbed in the pore are divided into "free water" having diffusion coefficients similar to those of bulk water at room temperature and "condensed water" which is about 10 times slower than bulk water owing to the interaction with the pore wall. The hydrogen atoms in the pore wall exhibited no relaxation within the measured time scales. The free water has, in the framework of the jump-diffusion model, smaller activation energy, longer residence time, and longer jump distance than bulk water. The neutron spin echo measurement revealed that the first order transition is a kind of liquid-liquid transition at which the free water is condensed on the pore surface in the low temperature phase. On cooling the condensed water, the relaxation time starts to deviate from the VFT equation around 200 K as previously observed in the water confined in nanoporous silicates. The free water plays an important role as the proton carrier but the proton conductivity is mainly governed by the number of protons provided into the adsorbed water from the pore wall. PMID:21999477
HZETRN: neutron and proton production in quasi-elastic scattering of GCR heavy-ions
NASA Technical Reports Server (NTRS)
Shavers, M. R.; Cucinotta, F. A.; Wilson, J. W.
2001-01-01
The development of transport models for radiation shielding design and evaluation has provided a series of deterministic computer codes that describe galactic cosmic radiation (GCR), solar particle events, and experimental beams at particle accelerators. These codes continue to be modified to accommodate new theory and improvements to the particle interaction database (Cucinotta et al., 1994, NASA Technical Paper 3472, US Government Printing Office, Washington DC). The solution employed by the heavy-ion transport code HZETRN was derived with the assumption that nuclear fragments are emitted with the same velocity as the incident ion through velocity conserving nuclear interactions. This paper presents a version of the HZETRN transport code that provides a more realistic distribution of the energy of protons and neutrons emitted from GCR interactions in shields. This study shows that the expected GCR dose equivalent is lower than previously calculated for water shields that are less than 110 g cm-2 thick. Calculations of neutron energy spectra in low Earth orbit indicate substantial contributions from relativistic neutrons. c2001 Elsevier Science Ltd. All rights reseved.
Microscopic properties of liquid gallium from quasi-elastic neutron scattering experiments
NASA Astrophysics Data System (ADS)
Blagoveshchenskii, N. M.; Novikov, A. G.; Puchkov, A. V.; Savostin, V. V.
2014-11-01
The results of the neutron diffraction study of liquid gallium on the DIN-2PI spectrometer (IBR-2 reactor, JINR, Dubna) have been discussed. The analysis of the experimental data has provided temperature dependences of diffusion and relaxation characteristics of liquid gallium in the temperature range of 313-793 K. It has been found that an increase in the temperature is accompanied by the gradual deviation of the temperature dependence of the self-diffusion coefficient from the known dependences obtained from the data on viscosity. Such a behavior is explained by the beginning clustering of liquid gallium induced by the prevailing covalent character of interatomic bonds.
[Inelastic electron scattering from surfaces]. [Progress report
Not Available
1993-10-01
This program uses ab-initio and multiple scattering to study surface dynamical processes; high-resolution electron-energy loss spectroscopy is used in particular. Off-specular excitation cross sections are much larger if electron energies are in the LEED range (50--300 eV). The analyses have been extended to surfaces of ordered alloys. Phonon eigenvectors and eigenfrequencies were used as inputs to electron-energy-loss multiple scattering cross section calculations. Work on low-energy electron and positron holography is mentioned.
Stimulated Electronic X-Ray Raman Scattering
NASA Astrophysics Data System (ADS)
Weninger, Clemens; Purvis, Michael; Ryan, Duncan; London, Richard A.; Bozek, John D.; Bostedt, Christoph; Graf, Alexander; Brown, Gregory; Rocca, Jorge J.; Rohringer, Nina
2013-12-01
We demonstrate strong stimulated inelastic x-ray scattering by resonantly exciting a dense gas target of neon with femtosecond, high-intensity x-ray pulses from an x-ray free-electron laser (XFEL). A small number of lower energy XFEL seed photons drive an avalanche of stimulated resonant inelastic x-ray scattering processes that amplify the Raman scattering signal by several orders of magnitude until it reaches saturation. Despite the large overall spectral width, the internal spiky structure of the XFEL spectrum determines the energy resolution of the scattering process in a statistical sense. This is demonstrated by observing a stochastic line shift of the inelastically scattered x-ray radiation. In conjunction with statistical methods, XFELs can be used for stimulated resonant inelastic x-ray scattering, with spectral resolution smaller than the natural width of the core-excited, intermediate state.
Chiral electron-chiral target scattering
Trantham, K.W.; Gay, T.J. Johnston, M.E.
1996-05-01
It is possible to have an electronic counterpart to the well known effect of optical circular dichroism: electron circular dichroism (ECD) is the preferential scattering of longitudinally polarized electrons by a chiral target. Resulting essentially from a difference in total scattering cross section for different incident electron helicities, this {open_quotes}parity-violating{close_quotes} effect is allowed by symmetry because the scattering target is handed. The authors have searched for ECD in camphor by measuring the transmitted intensity of electrons with positive (negative) helicity I{sub +({minus})} through a gas cell containing stereoisomers of camphor vapor and constructing the asymmetry A = (I{sub +} {minus} I{sub {minus}}). Within their sensitivity (2x10{sup {minus}4}) the authors were not able to detect ECD at the energies investigated (10 eV). Prospects for future investigations, particularly in light of the recent positive results measured in Muenster, will be discussed.
Pygmy Resonances Probed with Electron Scattering
Bertulani, Carlos A
2007-05-01
Pygmy resonances in light nuclei excited in electron scattering are discussed. These collective modes will be explored in future electron-ion colliders such as ELISe/FAIR (spokesperson: Haik Simon - GSI). Response functions for direct breakup are explored with few-body and hydrodynamical models, including the dependence upon final-state interactions.
Scattering of twisted relativistic electrons by atoms
NASA Astrophysics Data System (ADS)
Serbo, V.; Ivanov, I. P.; Fritzsche, S.; Seipt, D.; Surzhykov, A.
2015-07-01
The Mott scattering of high-energetic twisted electrons by atoms is investigated within the framework of the first Born approximation and Dirac's relativistic equation. Special emphasis is placed on the angular distribution and longitudinal polarization of the scattered electrons. In order to evaluate these angular and polarization properties we consider two experimental setups in which the twisted electron beam collides with either a single well-localized atom or macroscopic atomic target. Detailed relativistic calculations have been performed for both setups and for the electrons with kinetic energy from 10 to 1000 keV. The results of these calculations indicate that the emission pattern and polarization of outgoing electrons differ significantly from the scattering of plane-wave electrons and can be very sensitive to the parameters of the incident twisted beam. In particular, it is shown that the angular- and polarization-sensitive Mott measurements may reveal valuable information about both the transverse and longitudinal components of the linear momentum and the projection of the total angular momentum of twisted electron states. Thus, the Mott scattering emerges as a diagnostic tool for the relativistic vortex beams.
Mayer, Nathan Samuel
2011-12-05
The Main Injector Neutrino Oscillation Search (MINOS) is a two detector, long baseline neutrino oscillation experiment. The MINOS near detector is an ironscintillator tracking/sampling calorimeter and has recorded the world’s largest data set of neutrino interactions in the 0-5 GeV region. This high statistics data set is used to make precision measurements of neutrino interaction cross-sections on iron. The Q^{2} dependence in charged current quasi-elastic (CCQE) scattering probes the axial and vector structure (form factor) of the nucleon/nuclear target, and nuclear effects in neutrino scattering. Presented here is a study of the MINOS Data that will introduce a method that improves the existing MINOS CCQE analysis. This analysis uses an additional CCQE dominated sub-sample from a different kinematic region to reduce correlations between fit parameters in the existing MINOS CCQE analysis. The measured value of the axial-vector mass is M^{QE} _{A} = 1.312^{+0.037} _{-0.038}(fit)^{+0.123} _{-0.265}(syst.) GeV.
Zamrun, Muhammad; Usman, Ida; Variani, Viska Inda; Kassim, Hasan Abu
2014-03-05
We study the heavy-ion collision at sub-barrier energies of {sub 16}O+{sub 144}Sm system using full order coupled-channels formalism. We especially investigate the sensitivity of fusion and quasi-elastic barrier distributions for this system on the coupling radius parameter. We found that the coupled-channels calculations of the fusion and the quasi-elastic barrier distributions are sensitive to the coupling radius for this reaction in contrast to the fusion and quasi-elastic cross section. Our study indicates that the larger coupling radius, i.e., r{sub coup}=1.20, is required by the experimental quasi-elastic barrier distribution. However, the experimental fusion barrier distribution compulsory the small value, i.e., r{sub coup}=1.06.
Rotational rainbows in electron-molecule scattering
Ziegler, G.; Raedle, M.; Puetz, O.; Jung, K.; Ehrhardt, H.; Bergmann, K.
1987-06-22
We report the measurement of state-to-state differential cross sections for rotationally inelastic electron-Na/sub 2/ collisions for impact energies from 150 to 300 eV. The data demonstrate for the first time large rotational transitions (0less than or equal to..delta..jless than or equal to30) for backward scattering. The most surprising result is the observation of pronounced rotational rainbows. These structures are expected to be general features in high-energy electron-molecule scattering.
Electron scattering from silicon 30. Master's thesis
Bernhardt, G.P. IV
1983-01-01
In 1940, the first experiments on electron excitation of nuclei to discrete levels were done by Collins and Waldman. The first theoretical discussions of this inelastic electron scattering were due to Mamasachlisor in 1943 and Snedden and Touschek in 1948. Lyman et al. in 1951, using a betatron, clearly saw effects due to deviations from point Coulomb scattering, thus allowing nuclear sizes to be measured using electron elastic scattering. Since that time, linear accelerators have become the standard source of high-energy electrons for such work. However, due to the limited resolution, an experiment of the type done in this thesis was not possible before the current generation of linear accelerators and spectrometers. The machine used in the 1950's allowed electron scattering with a resolution of delta p/p 3/5x10 and with currents of a few tenths of a microampre. Work done using these machines, although including some excellent work such as that done by Hofstadter was limited to a few nuclei with well-isolated levels due to inability to resolve closely spaced levels.
Elastic electron scattering by ethyl vinyl ether
Khakoo, M. A.; Hong, L.; Kim, B.; Winstead, C.; McKoy, V.
2010-02-15
We report measured and calculated results for elastic scattering of low-energy electrons by ethyl vinyl ether (ethoxyethene), a prototype system for studying indirect dissociative attachment processes that may play a role in DNA damage. The integral cross section displays the expected {pi}{sup *} shape resonance. The agreement between the calculated and measured cross sections is generally good.
Multiple electron scattering routines for PEREGRINE
White, J A
1999-08-23
The Monte Carlo electron scattering routines solve multiple elastic scatters in a condensed history approach. The Goudsmit-Saunderson scattering model is used and its implementation is taken from Kawrakow and Bielajew[l]. The subroutines produce an exit angle representing a likely scattering angle of a single incident electron after scattering elastically over a given step size. Two input parameters, {lambda} and {eta}, that depend on the atomic species and incident energy must first be specified. The mapping from species and energy to 77 and {lambda} already existed in the PEREGRINE code and was not redone or modified in any way. The software has been validated by comparisons to Moliere and Goudsmit-Saunderson models of D.W.O. Rogers[2]. As required by licensing considerations, no public domain or copyrighted software has been used in any phase of the preparation of any of these sub-routines or data files. Apart from needing to have {eta} and {lambda} specified through PEREGRINE, the code provided is completely self-contained. Everything is written in the FORTRAN 77 language to simplify inclusion in the existing PEREGRINE package.
New Results from MiniBooNE Charged-Current Quasi-Elastic Anti-Neutrino Data
Grange, Joseph
2011-07-01
MiniBooNE anti-neutrino charged-current quasi-elastic (CCQE) data is compared to model predictions. The main background of neutrino-induced events is examined first, where three independent techniques are employed. Results indicate the neutrino flux is consistent with a uniform reduction of {approx}20% relative to the largely uncertain prediction. After background subtraction, the Q{sup 2} shape of {bar v}{sub {mu}} CCQE events is consistent with the model parameter MA = 1.35 GeV determined from MiniBooNE v{sub {mu}} CCQE data, while the normalization is {approx} 20% high compared to the same prediction.
Nonlinear wave scattering and electron beam relaxation
NASA Technical Reports Server (NTRS)
Muschietti, L.; Dum, C. T.
1991-01-01
The role played by nonlinear scattering during the relaxation of a warm electron beam is investigated through a numerical code based on kinetic equations. The code encompasses the quasi-linear wave-electron interaction and wave-wave scattering off ion clouds. Ions with velocities 2 nu sub i (nu sub i being the ion thermal velocity) are found to be the most efficient for scattering the Langmuir waves off their polarization clouds. The transfer rate of the spectrum out of resonance with the beam is larger by a factor 3 compared to usual estimates. The changes produced in the dispersion relation by the presence of the beam electrons dramatically alter the characteristics of the secondary spectrum. In a late phase the classic condensate K of about 0 is depleted, with the formation of a new condensate in resonance with the flat-topped beam distribution, which follows from the fact that the mere presence of the beam electrons creates a minimum in the frequency-wave-number relation. For strong and slow beams, the predictions of the code are found to be in excellent agreement with the results of the particle simulation if a dispersion relation that includes the beam is used.
Low Energy Electron Scattering from Fuels
NASA Astrophysics Data System (ADS)
Lopes, M. C. A.; Silva, D. G. M.; Bettega, M. H. F.; da Costa, R. F.; Lima, M. A. P.; Khakoo, M. A.; Winstead, C.; McKoy, V.
2012-11-01
In order to understand and optimize processes occurring during the ignition of plasma and its consequences in post-discharge for an internal combustion engine, especially considering the spark plug, we have produced in this work some basic information necessary to modeling spark ignition in alcohol- fuelled engines. Total cross sections of electron scattering by methanol and ethanol molecules in the energy range from 60 to 500 eV are reported, using the linear transmission method based on the Beer-Lambert law to first approximation. Aditionally to that, measurements and calculations of differential cross sections for elastic low-energy (rotationally unresolved) electron scattering were also discussed, for impact energies of 1, 2, 5, 10, 15, 20, 30, 50, and 100 eV and for scattering angles of 5°-130°. The measurements were obtained using the relative flow method with an aperture source, and calculations using two different implementations of the Schwinger multichannel method, one that takes all electrons into account and is adapted for parallel computers, and another that uses pseudopotentials and considers only the valence electrons.
SciNOvA: A Measurement of Neutrino-Nucleus Scattering in a Narrow-Band Beam
Paley, J.; Djurcic, Z.; Harris, D.; Tesarek, R.; Feldman, G.; Corwin, L.; Messier, M.D.; Mayer, N.; Musser, J.; Paley, J.; Tayloe, R.; /Indiana U. /Iowa State U. /Minnesota U. /South Carolina U. /Wichita State U. /William-Mary Coll.
2010-10-15
We propose to construct and deploy a fine-grained detector in the Fermilab NOvA 2 GeV narrow-band neutrino beam. In this beam, the detector can make unique contributions to the measurement of quasi-elastic scattering, neutral-current elastic scattering, neutral-current {pi}{sup 0} production, and enhance the NOvA measurements of electron neutrino appearance. To minimize cost and risks, the proposed detector is a copy of the SciBar detector originally built for the K2K long baseline experiment and used recently in the SciBooNE experiment.
Quark-Hadron Duality in Electron Scattering
W. Melnitchouk
2000-09-01
Quark-hadron duality addresses some of the most fundamental issues in strong interaction physics, in particular the nature of the transition from the perturbative to non-perturbative regions of QCD. I summarize recent developments in quark-hadron duality in lepton-hadron scattering, and outline how duality can be studied at future high-luminosity facilities such as Jefferson Lab at 12 GeV, or an electron-hadron collider such as EPIC.
Inelastic Scattering Of Electrons By Protons
DOE R&D Accomplishments Database
Cone, A. A.; Chen, K. W.; Dunning, J. R. Jr.; Hartwig, G.; Ramsey, N. F.; Walker, J. K.; Wilson, R.
1966-12-01
The inelastic scattering of electrons by protons has been measured at incident electron energies up to 5 BeV/c and momentum transfers q{sup 2}=4(BeV/c){sup 2}. Excitation of known nucleon resonances at M=1238, 1512, 1688 and possibly 1920 MeV have been observed. The calculations for the resonance at M=1238 MeV have been compared with calculations by Adler based on the dispersion theory of Chew, Goldberger, Low and Nambu. The agreement is good. Qualitative models are discussed for the other resonances.
Proton radius from electron scattering data
NASA Astrophysics Data System (ADS)
Higinbotham, Douglas W.; Kabir, Al Amin; Lin, Vincent; Meekins, David; Norum, Blaine; Sawatzky, Brad
2016-05-01
Background: The proton charge radius extracted from recent muonic hydrogen Lamb shift measurements is significantly smaller than that extracted from atomic hydrogen and electron scattering measurements. The discrepancy has become known as the proton radius puzzle. Purpose: In an attempt to understand the discrepancy, we review high-precision electron scattering results from Mainz, Jefferson Lab, Saskatoon, and Stanford. Methods: We make use of stepwise regression techniques using the F test as well as the Akaike information criterion to systematically determine the predictive variables to use for a given set and range of electron scattering data as well as to provide multivariate error estimates. Results: Starting with the precision, low four-momentum transfer (Q2) data from Mainz (1980) and Saskatoon (1974), we find that a stepwise regression of the Maclaurin series using the F test as well as the Akaike information criterion justify using a linear extrapolation which yields a value for the proton radius that is consistent with the result obtained from muonic hydrogen measurements. Applying the same Maclaurin series and statistical criteria to the 2014 Rosenbluth results on GE from Mainz, we again find that the stepwise regression tends to favor a radius consistent with the muonic hydrogen radius but produces results that are extremely sensitive to the range of data included in the fit. Making use of the high-Q2 data on GE to select functions which extrapolate to high Q2, we find that a Padé (N =M =1 ) statistical model works remarkably well, as does a dipole function with a 0.84 fm radius, GE(Q2) =(1+Q2/0.66 GeV2) -2 . Conclusions: Rigorous applications of stepwise regression techniques and multivariate error estimates result in the extraction of a proton charge radius that is consistent with the muonic hydrogen result of 0.84 fm; either from linear extrapolation of the extremely-low-Q2 data or by use of the Padé approximant for extrapolation using a larger
Future of Electron Scattering and Diffraction
Hall, Ernest; Stemmer, Susanne; Zheng, Haimei; Zhu, Yimei; Maracas, George
2014-02-25
The ability to correlate the atomic- and nanoscale-structure of condensed matter with physical properties (e.g., mechanical, electrical, catalytic, and optical) and functionality forms the core of many disciplines. Directing and controlling materials at the quantum-, atomic-, and molecular-levels creates enormous challenges and opportunities across a wide spectrum of critical technologies, including those involving the generation and use of energy. The workshop identified next generation electron scattering and diffraction instruments that are uniquely positioned to address these grand challenges. The workshop participants identified four key areas where the next generation of such instrumentation would have major impact: A – Multidimensional Visualization of Real Materials B – Atomic-scale Molecular Processes C – Photonic Control of Emergence in Quantum Materials D – Evolving Interfaces, Nucleation, and Mass Transport Real materials are comprised of complex three-dimensional arrangements of atoms and defects that directly determine their potential for energy applications. Understanding real materials requires new capabilities for three-dimensional atomic scale tomography and spectroscopy of atomic and electronic structures with unprecedented sensitivity, and with simultaneous spatial and energy resolution. Many molecules are able to selectively and efficiently convert sunlight into other forms of energy, like heat and electric current, or store it in altered chemical bonds. Understanding and controlling such process at the atomic scale require unprecedented time resolution. One of the grand challenges in condensed matter physics is to understand, and ultimately control, emergent phenomena in novel quantum materials that necessitate developing a new generation of instruments that probe the interplay among spin, charge, orbital, and lattice degrees of freedom with intrinsic time- and length-scale resolutions. Molecules and soft matter require imaging and
Electron scattering and transport in liquid argon
Boyle, G. J.; Cocks, D. G.; White, R. D.; McEachran, R. P.
2015-04-21
The transport of excess electrons in liquid argon driven out of equilibrium by an applied electric field is revisited using a multi-term solution of Boltzmann’s equation together with ab initio liquid phase cross-sections calculated using the Dirac-Fock scattering equations. The calculation of liquid phase cross-sections extends previous treatments to consider multipole polarisabilities and a non-local treatment of exchange, while the accuracy of the electron-argon potential is validated through comparison of the calculated gas phase cross-sections with experiment. The results presented highlight the inadequacy of local treatments of exchange that are commonly used in liquid and cluster phase cross-section calculations. The multi-term Boltzmann equation framework accounting for coherent scattering enables the inclusion of the full anisotropy in the differential cross-section arising from the interaction and the structure factor, without an a priori assumption of quasi-isotropy in the velocity distribution function. The model, which contains no free parameters and accounts for both coherent scattering and liquid phase screening effects, was found to reproduce well the experimental drift velocities and characteristic energies.
Electron scattering and transport in liquid argon.
Boyle, G J; McEachran, R P; Cocks, D G; White, R D
2015-04-21
The transport of excess electrons in liquid argon driven out of equilibrium by an applied electric field is revisited using a multi-term solution of Boltzmann's equation together with ab initio liquid phase cross-sections calculated using the Dirac-Fock scattering equations. The calculation of liquid phase cross-sections extends previous treatments to consider multipole polarisabilities and a non-local treatment of exchange, while the accuracy of the electron-argon potential is validated through comparison of the calculated gas phase cross-sections with experiment. The results presented highlight the inadequacy of local treatments of exchange that are commonly used in liquid and cluster phase cross-section calculations. The multi-term Boltzmann equation framework accounting for coherent scattering enables the inclusion of the full anisotropy in the differential cross-section arising from the interaction and the structure factor, without an a priori assumption of quasi-isotropy in the velocity distribution function. The model, which contains no free parameters and accounts for both coherent scattering and liquid phase screening effects, was found to reproduce well the experimental drift velocities and characteristic energies. PMID:25903897
Electron-helium scattering in Debye plasmas
Zammit, Mark C.; Fursa, Dmitry V.; Bray, Igor; Janev, R. K.
2011-11-15
Electron-helium scattering in weakly coupled hot-dense (Debye) plasma has been investigated using the convergent close-coupling method. The Yukawa-type Debye-Hueckel potential has been used to describe plasma Coulomb screening effects. Benchmark results are presented for momentum transfer cross sections, excitation, ionization, and total cross sections for scattering from the ground and metastable states of helium. Calculations cover the entire energy range up to 1000 eV for the no screening case and various Debye lengths (5-100 a{sub 0}). We find that as the screening interaction increases, the excitation and total cross sections decrease, while the total ionization cross sections increase.
P-Wave Electron-Hydrogen Scattering
NASA Technical Reports Server (NTRS)
Bhtia, Anand
2012-01-01
A variational wave function incorporating short range correlations via Hylleraas type functions plus long-range polarization terms of the polarized orbital type but with smooth cut-off factors has been used to calculate P-wave phase shifts for electron-hydrogen scattering. This approach gives the direct r(exp -4) potential and a non-local optical potential which is definite. The resulting phase shifts have rigorous lower bounds and the convergence is much faster than those obtained without the modification of the target function. Final results will be presented at the conference.
Dispersion corrections to parity violating electron scattering
Gorchtein, M.; Horowitz, C. J.; Ramsey-Musolf, M. J.
2010-08-04
We consider the dispersion correction to elastic parity violating electron-proton scattering due to {gamma}Z exchange. In a recent publication, this correction was reported to be substantially larger than the previous estimates. In this paper, we study the dispersion correction in greater detail. We confirm the size of the disperion correction to be {approx}6% for the QWEAK experiment designed to measure the proton weak charge. We enumerate parameters that have to be constrained to better than relative 30% in order to keep the theoretical uncertainty for QWEAK under control.
Scattering of electrons from neon atoms
NASA Technical Reports Server (NTRS)
Dasgupta, A.; Bhatia, A. K.
1984-01-01
Scattering of electrons from neon atoms is investigated by the polarized-orbital method. The perturbed orbitals calculated with use of the Sternheimer approximation lead to the polarizability 2.803 a(0)-cube in fairly good agreement with the experimental value 2.66 a(0)-cube. Phase shifts for various partial waves are calculated in the exchange, exchange-adiabatic, and polarized-orbital approximations. They are compared with the previous results. The calculated elastic differential, total, and momentum-transfer cross sections are compared with the experimental results. The polarized-orbital approximation yields results which show general improvement over the exchange-adiabatic approximation.
Electronic Raman scattering as a probe of anisotropic electron pairing
Devereaux, T.P.
1995-08-01
A theory for the electronic contribution to Raman scattering in anisotropic superconductors is presented. It is shown that Raman scattering can provide a wealth of polarization-(symmetry-) dependent information which probes the detailed angular dependence of the energy gap. Using a model band structure, the symmetry-dependent Raman spectra are calculated for d{sub x{sup 2}{minus}y{sup 2}} pairing and compared to the data taken on Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8}. Favorable agreement with the symmetry-dependent electronic spectra is shown. Further, the impurity dependence of theory is calculated, which provides an unique test of d{sub x{sup 2}{minus}y{sup 2}} pairing.
Inelastic electron scattering from a moving nucleon
Kuhn, S.E.; Griffioen, K.
1994-04-01
The authors propose to measure inelastically scattered electrons in coincidence with spectator protons emitted backwards relative to the virtual photon direction in the reaction d(e, e{prime}p{sub s})X. In a simple spectator model, the backward proton has equal and opposite momentum to the neutron before it is struck, allowing the authors to study the dependence on kinematics and off-shell behaviour of the electron-nucleon inelastic cross section. If the photon couples to a quark in a 6-quark bag, a different dependence of the cross section on the kinematic variables (x, Q{sup 2}, and p{sub s}) can be observed. This proposed experiment requires large acceptance and beam energies above 6 GeV. It is ideally suited for the CEBAF Large Acceptance Spectrometer (CLAS).
A Measurement of the Exclusive 3He(e,e'p) Reaction Below the Quasi-Elastic Peak
Kozlov, A; Sarty, A J; Aniol, K A; Bartsch, P; Baumann, D; Bertozzi, W; Bohinc, K; Bahm, R; Chen, J P; Dale, D; Dennis, L; Derber, S; Ding, M; Distler, M O; Dragovitsch, P; Ewald, I; Fissum, K G; Friedrich, J; Friedrich, J M; Geiges, R; Gilad, S; Jennewein, P; Kahrau, M; Kohl, M; Krygier, K W; Liesenfeld, A; Margaziotis, D J; Merkel, H; Merle, P; Moeller, U; Neuhausen, R; Pospischil, T; Potokar, M; Riccardi, G; Rochoe, R; Rosner, G; Rowntree, D; Schmieden, H; irca, S; Templon, J A; Thompson, M N; Wagner, A; Walcher, Th; Weis, M; Zhao, J; Zhou, Z -L; Golak, J; Glaeckle, W; Wita, H
2004-09-01
New, high-precision measurements of the 3He(e,e'p) reaction using the A1 collaboration spectrometers at the Mainz microtron MAMI are presented. These were performed in antiparallel kinematics at energy transfers below the quasi-elastic peak, and at a central momentum transfer of 685 MeV/c. Cross sections and distorted momentum distributions were extracted and compared to theoretical predictions and existing data. The longitudinal and transverse behavior of the cross section was also studied. Sizable differences in the cross-section behavior from theoretical predictions based on Plane Wave Impulse Approximation were observed in both the two- and three-body breakup channels. Full Faddeev-type calculations account for some of the observed excess cross section, but significant differences remain.
Novel internal target for electron scattering off unstable nuclei.
Wakasugi, M; Emoto, T; Furukawa, Y; Ishii, K; Ito, S; Koseki, T; Kurita, K; Kuwajima, A; Masuda, T; Morikawa, A; Nakamura, M; Noda, A; Ohnishi, T; Shirai, T; Suda, T; Takeda, H; Tamae, T; Tongu, H; Wang, S; Yano, Y
2008-04-25
A novel internal target has been developed, which will make electron scattering off short-lived radioactive nuclei possible in an electron storage ring. An "ion trapping" phenomenon in the electron storage ring was successfully utilized for the first time to form the target for electron scattering. Approximately 7 x 10(6) stable 133Cs ions were trapped along the electron beam axis for 85 ms at an electron beam current of 80 mA. The collision luminosity between the stored electrons and trapped Cs ions was determined to be 2.4(8) x 10(25) cm(-2) s(-1) by measuring elastically scattered electrons. PMID:18518208
Inelastic electron scattering on C{sub 60} clusters
Yabana, K.; Bertsch, G.F.
1993-12-31
We calculate the electronic excitation of C{sub 60} by inelastic electron scattering or electron energy loss spectroscopy (EELS). The scattering process is treated in the distorted-wave Born approximation, and the electronic excitations are calculated in a spherical basis model. We find that low energy electrons excite some non-photoactive modes, in agreement with experiment. Spin triplet modes are poorly excited, even at the lowest electron energies.
Quark-Hadron Duality in Electron Scattering
Wally Melnitchouk; Rolf Ent; Cynthia Keppel
2004-08-01
The duality between partonic and hadronic descriptions of physical phenomena is one of the most remarkable features of strong interaction physics. A classic example of this is in electron-nucleon scattering, in which low-energy cross sections, when averaged over appropriate energy intervals, are found to exhibit the scaling behavior expected from perturbative QCD. We present a comprehensive review of data on structure functions in the resonance region, from which the global and local aspects of duality are quantified, including its flavor, spin and nuclear medium dependence. To interpret the experimental findings, we discuss various theoretical approaches which have been developed to understand the microscopic origins of quark-hadron duality in QCD. Examples from other reactions are used to place duality in a broader context, and future experimental and theoretical challenges are identified.
Two-photon exchange in electron-trinucleon elastic scattering
NASA Astrophysics Data System (ADS)
Kobushkin, A. P.; Timoshenko, Ju. V.
2013-10-01
We discuss two-photon exchange (TPE) in elastic electron scattering off the trinucleon systems, 3He and 3H. The calculations are done in the semirelativistic approximation with the trinucleon wave functions obtained with the Paris and CD-Bonn nucleon-nucleon potentials. An applicability area of the model is wide enough and includes the main part of kinematical domain where experimental data exist. All three TPE amplitudes (generalized form factors) for electron 3He elastic scattering are calculated. We find that the TPE amplitudes are a few times more significant in the scattering of electrons off 3He then in the electron-proton scattering.
Fingerprints of Multiple Electron Scatterings in Single-Layer Graphene
NASA Astrophysics Data System (ADS)
Jung, Minbok; Sohn, So-Dam; Park, Jonghyun; Lee, Keun-U.; Shin, Hyung-Joon
2016-03-01
The electrons in graphene exhibit unusual behaviours, which can be described by massless Dirac quasiparticles. Understanding electron scattering in graphene has been of significant importance for its future application in electronic devices because electron scattering determines electrical properties such as resistivity and electron transport. There are two types of electron scatterings in graphene: intervalley scattering and intravalley scattering. In single-layer graphene, to date, it has been difficult to observe intravalley scattering because of the suppression of backscattering resulting from the chiral nature of the electrons in graphene. Here, we report the multiple electron scattering behaviours in single-layer graphene on a metallic substrate. By applying one- and two-dimensional Fourier transforms to maps of the local density of states, we can distinguish individual scattering processes from complex interference patterns. These techniques enable us to provide direct evidence of intravalley scattering, revealing a linear dispersion relation with a Fermi velocity of ~7.4 × 105 m/s.
No surprise in the first Born approximation for electron scattering.
Lentzen, M
2014-01-01
In a recent article it is argued that the far-field expansion of electron scattering, a pillar of electron diffraction theory, is wrong (Treacy and Van Dyck, 2012). It is further argued that in the first Born approximation of electron scattering the intensity of the electron wave is not conserved to first order in the scattering potential. Thus a "mystery of the missing phase" is investigated, and the supposed flaw in scattering theory is seeked to be resolved by postulating a standing spherical electron wave (Treacy and Van Dyck, 2012). In this work we show, however, that these theses are wrong. A review of the essential parts of scattering theory with careful checks of the underlying assumptions and limitations for high-energy electron scattering yields: (1) the traditional form of the far-field expansion, comprising a propagating spherical wave, is correct; (2) there is no room for a missing phase; (3) in the first Born approximation the intensity of the scattered wave is conserved to first order in the scattering potential. The various features of high-energy electron scattering are illustrated by wave-mechanical calculations for an explicit target model, a Gaussian phase object, and for a Si atom, considering the geometric conditions in high-resolution transmission electron microscopy. PMID:24216157
Fingerprints of Multiple Electron Scatterings in Single-Layer Graphene
Jung, Minbok; Sohn, So-Dam; Park, Jonghyun; Lee, Keun-U; Shin, Hyung-Joon
2016-01-01
The electrons in graphene exhibit unusual behaviours, which can be described by massless Dirac quasiparticles. Understanding electron scattering in graphene has been of significant importance for its future application in electronic devices because electron scattering determines electrical properties such as resistivity and electron transport. There are two types of electron scatterings in graphene: intervalley scattering and intravalley scattering. In single-layer graphene, to date, it has been difficult to observe intravalley scattering because of the suppression of backscattering resulting from the chiral nature of the electrons in graphene. Here, we report the multiple electron scattering behaviours in single-layer graphene on a metallic substrate. By applying one- and two-dimensional Fourier transforms to maps of the local density of states, we can distinguish individual scattering processes from complex interference patterns. These techniques enable us to provide direct evidence of intravalley scattering, revealing a linear dispersion relation with a Fermi velocity of ~7.4 × 105 m/s. PMID:26936521
Electron Scattering by biomass molecular fragments
NASA Astrophysics Data System (ADS)
Lima, Marco
2015-09-01
The replacement of fossil fuels by biofuels from renewable sources may not be a definite answer for greenhouse gas emissions problems, but it is a good step towards a sustainable energy strategy. Few per cent of ethanol is being mixed to gasoline in many countries and in some of them, like Brazil, a very aggressive program has been developed, using, in large scale, flex fuel engines that can run with any mixture of gasoline and ethanol, including 100% ethanol. Important points are how to produce ethanol in a sustainable way and with which technology? Biomass is a good candidate to enhance the first generation (produced from Corn in USA and from sugarcane in Brazil) production towards the so-called second-generation ethanol, since it has cellulose and hemicellulose as source of sugars. In order to liberate these sugars for fermentation, it is important to learn how to separate the main components. Chemical routes (acid treatment) and biological routes (enzymatic hydrolysis) are combined and used for these purposes. Atmospheric plasmas can be useful for attacking the biomass in a controlled manner and low energy electrons may have an important role in the process. Recently, we have been studying the interaction of electrons with lignin subunits (phenol, guaiacol, p-coumaryl alcohol), cellulose components, β-D-glucose and cellobiose (β(1-4) linked glucose dimer) and hemicellulose components [2] (β-D-xylose). We also obtained results for the amylose subunits α-D-glucose and maltose (α(1-4) linked glucose dimer). Altogether, the resonance spectra of lignin, cellulose and hemicellulose components establish a physical-chemical basis for electron-induced biomass pretreatment that could be applied to biofuel production. In order to describe a more realistic system (where molecules are ``wet''), we have obtained the shape resonance spectra of phenol-water clusters, as obtained previously from elastic electron scattering calculations. Our results, obtained in a simple
Laser-induced resonant structure in electron-atom scattering
NASA Astrophysics Data System (ADS)
Flegel, A. V.; Frolov, M. V.; Manakov, N. L.; Starace, Anthony F.
2009-11-01
Orders of magnitude increases are predicted in the cross sections for electron-atom scattering accompanied by absorption or emission of n laser photons for incident electron energies at which the electron, by emitting μ laser photons, can be captured by the atom to form a negative ion. Resonance enhancements are most significant in the plateau region (n gg μ) of the scattered electron spectrum, whose shape is predicted to replicate that of the ion's (n + μ)-photon detachment spectrum.
Electron impact elastic scattering and vibrational excitation of ethylene
NASA Astrophysics Data System (ADS)
Khakoo, Murtadha; Khakoo, Sabaha; Sakaamini, Ahmad; Hargreaves, Leigh; Winstead, Carl; McKoy, Vince
2015-09-01
Experimental and theoretical (Schwinger Multi-Channel model) differential scattering cross sections for low energy electron elastic scattering plus vibrational excitation (4 energy loss features) of ethylene are presented. The incident electron energy range is from 0.5eV to 100eV and scattering angles of 5 to 130 degrees. Comparisons with theory and past available measurements show good agreement in general. Funded by a National Science Foundation Collaborative Research Grant to CSUF and Caltech.
Electron Elastic-Scattering Cross-Section Database
National Institute of Standards and Technology Data Gateway
SRD 64 NIST Electron Elastic-Scattering Cross-Section Database (PC database, no charge) This database provides values of differential elastic-scattering cross sections, corresponding total elastic-scattering cross sections, phase shifts, and transport cross sections for elements with atomic numbers from 1 to 96 and for electron energies between 50 eV and 20,000 eV (in steps of 1 eV).
Polarized electron scattering, new physics and dark parity violation
Marciano, William J.
2013-11-07
'New Physics' sensitivities of polarized electron scattering asymmetries, atomic parity violation, m{sub W} and sin{sup 2} θ{sub W} (Z pole measurements) are compared. The utility of low Q{sup 2} polarized electron scattering for probing parity violating 'dark boson' effects is discussed. A possible determination of the weak charge Q{sub w}({sup 12}C) to about ±0.3% via elastic e-Carbon scattering is advocated.
Watabe, Masaki
2010-05-01
MINOS (Main Injector Neutrino Oscillation Search) experiment has been designed to search for a change in the avor composition of a beam of muon neutrinos as they travel between the Near Detector at Fermi National Accelerator Laboratory and the Far Detector in the Soudan mine in Minnesota, 735 km from the target. The MINOS oscillation analysis is mainly performed with the charged current (CC) events and sensitive to constrain high- Δm^{2} values. However, the quasi-elastic (QEL) charged current interaction is dominant in the energy region important to access low- m^{2} values. For further improvement, the QEL oscillation analysis is performed in this dissertation. A data sample based on a total of 2.50 x 10^{20} POT is used for this analysis. In summary, 55 QEL-like events are observed at the Far detector while 87.06 ± 13.17 (syst:) events are expected with null oscillation hypothesis. These data are consistent with disappearance via oscillation with m^{2} = 2:10 0.37 (stat:) ± 0.24 (syst:) eV^{2} and the maximal mixing angle.
Schwinger-Keldysh canonical formalism for electronic Raman scattering
NASA Astrophysics Data System (ADS)
Su, Yuehua
2016-03-01
Inelastic low-energy Raman and high-energy X-ray scatterings have made great progress in instrumentation to investigate the strong electronic correlations in matter. However, theoretical study of the relevant scattering spectrum is still a challenge. In this paper, we present a Schwinger-Keldysh canonical perturbation formalism for the electronic Raman scattering, where all the resonant, non-resonant and mixed responses are considered uniformly. We show how to use this formalism to evaluate the cross section of the electronic Raman scattering off an one-band superconductor. All the two-photon scattering processes from electrons, the non-resonant charge density response, the elastic Rayleigh scattering, the fluorescence, the intrinsic energy-shift Raman scattering and the mixed response, are included. In the mean-field superconducting state, Cooper pairs contribute only to the non-resonant response. All the other responses are dominated by the single-particle excitations and are strongly suppressed due to the opening of the superconducting gap. Our formalism for the electronic Raman scattering can be easily extended to study the high-energy resonant inelastic X-ray scattering.
Hottes, M. Muench, F.; Rauber, M.; Stegmann, C.; Ensinger, W.; Dassinger, F.; Schlaak, H. F.
2015-02-02
In this Letter, we describe the electrodeposition of capped, micro-sized Pt nanowire arrays in ion-track etched polymer templates and measure their collective mechanical response to an external force. By using an aperture mask during the irradiation process, it was possible to restrict the creation of pores in the templates to defined areas, allowing the fabrication of small nanowire arrays in different geometries and sizes. The simultaneous and highly reliable formation of many nanowire arrays was achieved using a pulsed electrodeposition technique. After deposition, the polymer matrix was removed using a gentle, dry oxygen plasma treatment, resulting in an excellent preservation of the array nanostructure as confirmed by scanning electron microscopy. A force measuring station was set up to perform mechanical characterization series on free-standing arrays. The nanowire arrays show a high robustness and respond sensitively to the applied force, making them attractive as spring elements in miniaturized inertial sensors, for example.
Recent progress in electron scattering from atoms and molecules
Brunger, M. J.; Buckman, S. J.; Sullivan, J. P.; Palihawadana, P.; Jones, D. B.; Chiari, L.; Pettifer, Z.; Silva, G. B. da; Lopes, M. C. A.; Duque, H. V.; Masin, Z.; Gorfinkiel, J. D.; Garcia, G.; Hoshino, M.; Tanaka, H.; Limão-Vieira, P.
2014-03-05
We present and discuss recent results, both experimental and theoretical (where possible), for electron impact excitation of the 3s[3/2 ]{sub 1} and 3s′[1/2 ]{sub 1} electronic states in neon, elastic electron scattering from the structurally similar molecules benzene, pyrazine, and 1,4-dioxane and excitation of the electronic states of the important bio-molecule analogue α-tetrahydrofurfuryl alcohol. While comparison between theoretical and experimental results suggests that benchmarked cross sections for electron scattering from atoms is feasible in the near-term, significant further theoretical development for electron-molecule collisions, particularly in respect to discrete excitation processes, is still required.
Electron scattering intensities and Patterson functions of Skyrmions
NASA Astrophysics Data System (ADS)
Karliner, M.; King, C.; Manton, N. S.
2016-06-01
The scattering of electrons off nuclei is one of the best methods of probing nuclear structure. In this paper we focus on electron scattering off nuclei with spin and isospin zero within the Skyrme model. We consider two distinct methods and simplify our calculations by use of the Born approximation. The first method is to calculate the form factor of the spherically averaged Skyrmion charge density; the second uses the Patterson function to calculate the scattering intensity off randomly oriented Skyrmions, and spherically averages at the end. We compare our findings with experimental scattering data. We also find approximate analytical formulae for the first zero and first stationary point of a form factor.
Collisionless pitch-angle scattering of runaway electrons
NASA Astrophysics Data System (ADS)
Liu, Jian; Wang, Yulei; Qin, Hong
2016-06-01
It is discovered that the tokamak field geometry generates a toroidicity induced broadening of the pitch-angle distribution of runaway electrons. This collisionless pitch-angle scattering is much stronger than the collisional scattering and invalidates the gyro-center model for runaway electrons. As a result, the energy limit of runaway electrons is found to be larger than the prediction of the gyro-center model and to depend heavily on the background magnetic field.
The effect of electron scattering redistribution on atomic line polarization
NASA Astrophysics Data System (ADS)
Supriya, H. D.; Nagendra, K. N.; Sampoorna, M.; Ravindra, B.
2012-09-01
The polarization of spectral lines is generated by the scattering of angularly anisotropic incident radiation field on the atoms in the stellar atmosphere. This atomic scattering polarization is modified by frequency non-coherent scattering of line photons on free electrons. With modern spectropolarimeters of high sensitivity, it is possible to detect such changes in the spectral line polarization caused by scattering on electrons. We present new and efficient numerical techniques to solve the problem of line radiative transfer with atomic and electron scattering frequency redistribution in planar media. The evaluation and use of angle-dependent partial frequency redistribution functions (both atomic and electron scattering type) in the transfer equation require a lot of computing effort. In this paper, we apply a decomposition technique to handle this numerically difficult problem. This recently developed technique is applied for the first time to the electron scattering partial redistribution. This decomposition technique allows us to devise fast iterative methods of solving the polarized line transfer equation. An approximate lambda iteration (ALI) method and a method based on Neumann series expansion of the polarized source vector are proposed. We show that these numerical methods can be used to obtain a solution of the problem, when both atomic and electron scattering partial frequency redistribution are considered together. This is in contrast with the classical numerical methods which require a great amount of computing time. We show the importance of electron scattering redistribution in the far wing line polarization, which has practical implications in the analysis of polarized stellar or solar spectra, where non-coherent electron scattering controls the line wing transfer.
The effects of density-dependent form factors for (e, e'p) reaction in quasi-elastic region
NASA Astrophysics Data System (ADS)
Kim, K. S.; Cheoun, Myung-Ki; Kim, Hungchong; So, W. Y.
2016-04-01
Within the framework of a relativistic single particle model, the effects of density-dependent electromagnetic form factors on the exclusive (e,e'p) reaction are investigated in the quasi-elastic region. The density-dependent electromagnetic form factors are generated from a quark-meson coupling model and used to calculate the cross sections in two different densities, either at the normal density of ρ_0 ˜ 0.15 fm^-3 or at the lower density, 0.5ρ_0 . Then these cross sections are analyzed in the two different kinematics: One is that the momentum of the outgoing nucleon is along the momentum transfer. The other is that the angle between the momentum of the outgoing nucleon and the momentum transfer is varied at fixed magnitude of the momentum of the outgoing nucleon. Our theoretical differential reduced cross sections are compared with the NIKHEF data for the 208 Pb( e, e'p) reaction, which is related to the probability that a bound nucleon from a given orbit can be knocked-out of the nucleus. The effects of the density-dependent form factors increase the differential cross sections for both knocked-out proton and neutron by an amount of a few percent. Moreover they are shown to be almost the same within only a few percent, i.e., nearly independent of the shell location of knockout nucleons. These results are quite consistent with the characteristics of double magic nuclei which have relatively sharp smearing in the density distribution.
Precision electroweak studies using parity violation in electron scattering
Paschke, Kent D,
2013-11-01
The nature of new neutral-current interactions can be revealed at the low-energy precision frontier, where studies of parity-violation in electron scattering will complement the energy-frontier studies at the LHC. Measurements of the parity-violating observable APV - the cross-section asymmetry in the scattering of longitudinally polarized electrons from an unpolarized target - are sensitive to possible contact interactions from new physics at multi-TeV mass scales. The 12 GeV upgrade at JLab and a new, high-intensity beam at Mainz offer opportunities for significant improvements in measurements of electron-electron and electron-quark parity-violating interactions.
Atmospheric scattering and decay of inner radiation belt electrons
NASA Astrophysics Data System (ADS)
Selesnick, R. S.
2012-08-01
The dynamics of inner radiation belt electrons are governed by competing source, loss, and transport processes. However, during the recent extended solar minimum period the source was inactive and electron intensity was characterized by steady decay. This provided an opportunity to determine contributions to the decay rate of losses by precipitation into the atmosphere and of diffusive radial transport. To this end, a stochastic simulation of inner radiation belt electron transport is compared to data taken by the IDP instrument on the DEMETER satellite during 2009. For quasi-trapped, 200 keV electrons atL= 1.3, observed in the drift loss cone (DLC), results are consistent with electron precipitation losses by atmospheric scattering alone, provided account is taken of non-diffusive wide-angle scattering. Such scattering is included in the stochastic simulation using a Markov jump process. Diffusive small-angle atmospheric scattering, while causing most of the precipitation losses, is too slow relative to azimuthal drift to contribute significantly to DLC intensity. Similarly there is no contribution from scattering by VLF plasma waves. Energy loss, energy diffusion, and azimuthal drift are also included in the model. Even so, observed decay rates of stably-trapped electrons withL < 1.5 are slower than predicted by scattering losses alone, requiring radial diffusion with coefficient DLL ˜ 3 × 10-10 s-1 to replenish electrons lost to the atmosphere at low L values.
Effect of multiple scattering on Cerenkov radiation from energetic electrons
Zheng Jian
2013-01-15
Cerenkov radiation can be used as a diagnostic tool to study energetic electrons generated in ultra-intense laser matter interactions. However, electrons suffer scattering with nuclei as they move in a medium. In this article, we theoretically study the effect of multiple scattering on Cerenkov radiation, and obtain analytical formulas under some circumstances. The results show that when the speed of an energetic electron is not close to the light speed in the medium, Cerenkov radiation is just slightly decreased due to multiple scattering. In the case that the electron speed is very close to the light speed in the medium, the effect of multiple scattering becomes significant, and the radiation is dominated by bremsstrahlung.
Multiple scattering of electrons in the reflex triode
Creedon, J.M. )
1990-12-01
Analytical theories and Monte Carlo calculations are used to treat the scattering and energy loss of electrons in the anode of a reflex triode. The solution of this scattering problem is combined with the equations for particle flow in vacuum to give a quantitative theory of triode operation. It is now possible to calculate several important properties of this device. These include the operating voltage in the constant voltage mode, the ratio of ion-to-electron current and the ion transit time.
Mettille, M.J.; Hester, R.D.
1988-05-01
Characterization of polymer molecular weight is an extremely important aspect of polymer research, and a vast number of analytical techniques has been used to determine molecular weights. One method is dynamic light scattering (DLS). DLS is also referred to as photon correlation spectroscopy (PCS), quasi-elastic light scattering (QLS), and may other appellations. The phenomenon that gives rise to the DLS technique was first observed in the early 1930's. In the mid 1950's, measurement techniques similar to modern dynamic light scattering were developed. Two major technical developments have greatly enhanced the use of DLS. The first was the development of the laser. This provided a light source with very high intensity at a single frequency. Also, major advances in digital electronics have allowed better data acquisition and faster data analysis than were previously available.
Parity Violation in Forward Angle Elastic Electron Proton Scattering
Krishna Kumar
1999-07-01
HAPPEX is a new experiment to probe the strange structure of the nucleon with parity violating electron scattering. We describe the physics motivation, provide an experimental overview and report on the results from the first data run. The asymmetry for the elastic scattering of 3.3 GeV electrons off target protons at a scattering angle of 12.5 degrees was measured to a precision of 15% of itself. The contribution from strange quark form factors was found to be zero within the experimental and theoretical uncertainties.
A discrete variable representation for electron-hydrogen atom scattering
NASA Astrophysics Data System (ADS)
Gaucher, Lionel Francis
1994-08-01
A discrete variable representation (DVR) suitable for treating the quantum scattering of a low energy electron from a hydrogen atom is presented. The benefits of DVR techniques (e.g. the removal of the requirement of calculating multidimensional potential energy matrix elements and the availability of iterative sparse matrix diagonalization/inversion algorithms) have for many years been applied successfully to studies of quantum molecular scattering. Unfortunately, the presence of a Coulomb singularity at the electrically unshielded center of a hydrogen atom requires high radial grid point densities in this region of the scattering coordinate, while the presence of finite kinetic energy in the asymptotic scattering electron also requires a sufficiently large radial grid point density at moderate distances from the nucleus. The constraints imposed by these two length scales have made application of current DVR methods to this scattering event difficult.
Spin relaxation in bilayer graphene: the role of electron-electron scattering
NASA Astrophysics Data System (ADS)
Katiyar, Saurabh; Ghosh, Bahniman; Salimath, Akshay Kumar
2016-02-01
This paper investigates the influence of electron-electron scattering on spin relaxation length in bilayer graphene using semiclassical Monte Carlo simulation. Both D'yakonov-P'erel and Elliot-Yafet mechanisms are considered for spin relaxation. It is shown that spin relaxation length decreases by 17 % at 300 K on including electron-electron scattering. The reason of this variation in spin relaxation length is that the ensemble spin is modified upon an e-e collision, and also e-e scattering rate is greater than phonon scattering rate which causes change in spin transport profile.
Effects of Auger electron elastic scattering in quantitative AES
NASA Astrophysics Data System (ADS)
Jablonski, Aleksander
1987-09-01
The Monte Carlo algorithm was developed for simulating the trajectories of electrons elastically scattered in the solid. The distribution of scattering angles was determined using the partial wave expansion method. This algorithm was used to establish the influence of Auger electron elastic collisions on the results of quantitative AES analysis. The calculations were performed for the most pronounced KLL, L 3 MM and M 5NN Auger transitions. It turned out that due to the elastic collisions the Auger electron signal is decreased by up to 10%. The corresponding decreased of the escape depth of Auger electrons reaches 30% as compared with the value derived from the inelastic mean free path. The values of the inelastic mean free path resulting from the overalyer method may be strongly affected by elastic scattering of Auger electrons.
Inverse Compton Scattering from Laser Accelerated Quasi-Monoenergetic Electrons
NASA Astrophysics Data System (ADS)
Mori, Yoshitaka; Kuwabara, Hajime; Ishii, Katsuhiro; Hanayama, Ryohei; Kawashima, Toshiyuki; Kitagawa, Yoneyoshi
2010-11-01
The progress of the laser accelerator shows us the possible applications to the industries, such as an inspection source for soft materials like as human bodies, plants foods and medicines. The inverse Compton scattering will realize such a novel inspection system. We demonstrate for the fist time that the laser-accelerated mono-energetic electrons inversely scatter the same counter laser beam to the Compton X-ray emissions. A Ti:sapphire laser (500mJ width 150fs) is divided into two beams. Main beam is focused to an edge of a helium gasjet to accelerate electrons to 13 and 22 MeV monoenergies, which inversely scattered the counter laser beam into 6 and 11 keV X-ray emissions in agreement with that calculated from the obtained electron spectra. The scattering is within 30 deg. around the main beam direction.
Path integral approach to electron scattering in classical electromagnetic potential
NASA Astrophysics Data System (ADS)
Chuang, Xu; Feng, Feng; Ying-Jun, Li
2016-05-01
As is known to all, the electron scattering in classical electromagnetic potential is one of the most widespread applications of quantum theory. Nevertheless, many discussions about electron scattering are based upon single-particle Schrodinger equation or Dirac equation in quantum mechanics rather than the method of quantum field theory. In this paper, by using the path integral approach of quantum field theory, we perturbatively evaluate the scattering amplitude up to the second order for the electron scattering by the classical electromagnetic potential. The results we derive are convenient to apply to all sorts of potential forms. Furthermore, by means of the obtained results, we give explicit calculations for the one-dimensional electric potential. Project supported by the National Natural Science Foundation of China (Grant Nos. 11374360, 11405266, and 11505285) and the National Basic Research Program of China (Grant No. 2013CBA01504).
The Quasi-Elastic Region of the IRON-56+IRON-56 and IRON-56+URANIUM-238 Reactions
NASA Astrophysics Data System (ADS)
Weston-Dawkes, Andrew Peter
Projectile-like fragments (PLF's) were detected for the 15-MeV/uFe+Fe and Fe+U reactions. The mass, charge and energy of the PLF's were recorded. For the Fe+Fe reaction light-charged particles were also recorded in coincidence with PLF's. Products with kinetic energies corresponding to the first 100 MeV of energy loss were studied in detail for a variety of questions that remain concerning the quasi -elastic region. PLF energy spectra clearly show the presence of structures. These structures can be classified as either narrow or broad in kinetic energy width. By use of evaporation calculations, it was shown that broad structures were due to normal evaporation processes. Narrow structures with widths of 8 to 10 MeV could not be duplicated by evaporation calculations and their origin is still unexplained. The evaporation peaks seen in the cobalt isotope energy spectra were used to determine the mean value of the excitation energy division (EED) since it was shown that this is the main determining factor in the value of the evaporation peak centroid. The results of the EED determinations indicate that many model assumptions of excitation energy division with nucleon exchange may be inapplicable during the first stages of interaction. The variance of the EED was determined for certain cobalt isotopes by use of an iteractive fitting program based on the evaporation process. For the 15-MeV/u systems it was found that the EED variance was smaller than what would be predicted by Morrissey's thermal variance. The optimum Q-values for cobalt isotopes were found to be effected by evaporation processes. After evaporation corrections to these values, it was found that Siemen's optimum Q-value model accurately predicted all values for the Fe+U system and most values for the Fe+Fe system. The exception was for the one proton transfer to ('57)Co in the Fe+Fe system, which has a much larger optimum Q-value than predicted. This may indicate a fundamental difference in proton
Surface roughness scattering of electrons in bulk mosfets
Zuverink, Amanda Renee
2015-11-01
Surface-roughness scattering of electrons at the Si-SiO_{2} interface is a very important consideration when analyzing Si metal-oxide-semiconductor field-effect transistors (MOSFETs). Scattering reduces the mobility of the electrons and degrades the device performance. 250-nm and 50-nm bulk MOSFETs were simulated with varying device parameters and mesh sizes in order to compare the effects of surface-roughness scattering in multiple devices. The simulation framework includes the ensemble Monte Carlo method used to solve the Boltzmann transport equation coupled with a successive over-relaxation method used to solve the two-dimensional Poisson's equation. Four methods for simulating the surface-roughness scattering of electrons were implemented on both devices and compared: the constant specularity parameter, the momentum-dependent specularity parameter, and the real-space-roughness method with both uniform and varying electric fields. The specularity parameter is the probability of an electron scattering speculariy from a rough surface. It can be chosen as a constant, characterizing partially diffuse scattering of all electrons from the surface the same way, or it can be momentum dependent, where the size of rms roughness and the normal component of the electron wave number determine the probability of electron-momentum randomization. The real-space rough surface method uses the rms roughness height and correlation length of an actual MOSFET to simulate a rough interface. Due to their charge, electrons scatter from the electric field and not directly from the surface. If the electric field is kept uniform, the electrons do not perceive the roughness and scatter as if from a at surface. However, if the field is allowed to vary, the electrons scatter from the varying electric field as they would in a MOSFET. These methods were implemented for both the 50-nm and 250-nm MOSFETs, and using the rms roughness heights and correlation lengths for real devices. The
Elastic scattering of electrons from Rb, Cs and Fr atoms
NASA Astrophysics Data System (ADS)
Gangwar, R. K.; Tripathi, A. N.; Sharma, L.; Srivastava, R.
2010-04-01
Differential, integrated elastic, momentum-transfer and total cross sections as well as differential S, T and U spin parameters for scattering of electrons from rubidium, caesium and francium atoms in the incident energy range up to 300 eV are calculated using a relativistic Dirac equation. The projectile electron-target atom interaction is represented by both real and complex parameter-free optical potentials for obtaining the solution of a Dirac equation for scattered electrons. The Dirac-Fock wavefunctions have been used to represent the Rb, Cs and Fr target atoms. The results of differential cross sections and spin asymmetry parameter S for e-Rb and e-Cs have been compared with the available experimental and theoretical results. Detailed results are reported for the elastic scattering of electrons from the ground states of a francium atom for the first time in the wide range of incident electron energies. The results of electron-Fr elastic scattering show the similar features to those obtained in the case of e-Rb and e-Cs elastic scattering.
Linden, Steven K.
2011-01-01
Charged current single pion production (CCπ^{+}) and charged current quasi-elastic scattering (CCQE) are the most abundant interaction types for neutrinos at energies around 1 GeV, a region of great interest to oscillation experiments. The cross-sections for these processes, however, are not well understood in this energy range. This dissertation presents a measurement of the ratio of CCπ^{+} to CCQE cross-sections for muon neutrinos on mineral oil (CH_{2}) in the MiniBooNE experiment. The measurement is presented here both with and without corrections for hadronic re-interactions in the target nucleus and is given as a function of neutrino energy in the range 0.4 GeV < E_{ν} < 2.4 GeV. With more than 46,000 CCπ^{+} events collected in MiniBooNE, and with a fractional uncertainty of roughly 11% in the region of highest statistics, this measurement represents a dramatic improvement in statistics and precision over previous CCπ^{+} and CCQE measurements.
Resonance formation in low energy electron scattering from uracil
NASA Astrophysics Data System (ADS)
Mašín, Zdeněk; Gorfinkiel, Jimena D.
2014-05-01
We present detailed ab initio results for resonance formation in low energy electron scattering from uracil obtained with the R-matrix method. We identify a larger number of resonances than any previous theoretical study. Most of these resonances have core-excited shape character and appear to be associated to the ring structure of the molecule. Their link to DEA spectra and to the resonances present in electron scattering from pyrimidine are discussed. Contribution to the Topical Issue "Electron and Positron Induced Processes", edited by Michael Brunger, Radu Campeanu, Masamitsu Hoshino, Oddur Ingólfsson, Paulo Limão-Vieira, Nigel Mason, Yasuyuki Nagashima and Hajime Tanuma.
Mott scattering of polarized electrons in a strong laser field
Manaut, B.; Taj, S.; Attaourti, Y.
2005-04-01
We present analytical and numerical results of the relativistic calculation of the transition matrix element S{sub fi} and differential cross sections for Mott scattering of initially polarized Dirac particles (electrons) in the presence of a strong laser field with linear polarization. We use exact Dirac-Volkov wave functions to describe the dressed electrons and the collision process is treated in the first Born approximation. The influence of the laser field on the degree of polarization of the scattered electron is reported.
Neutrino-electron scattering. Progress report
White, D.H.
1982-01-01
We present here a progress report on an experiment to measure the cross section for nu/sub ..mu../e scattering at the Brookhaven AGS. A wide band focussing horn is used with a neutrino beam energy centered at 1.5 GeV. We have in hand measurements with nu/sub ..mu../ and anti nu/sub ..mu../ beams but we present preliminary data on the nu/sub ..mu../ beam running only. We also measure the reactions: nu/sub ..mu../ + n ..-->.. ..mu../sup -/ + p and nu/sub e/ + n ..-->.. e/sup -/ + p which will be used in normalization and in background estimation.
Alonso, M. P.; Figueiredo, A. C. A.; Berni, L. A.; Machida, M.
2010-10-15
We present the first simultaneous measurements of the Thomson scattering and electron cyclotron emission radiometer diagnostics performed at TCABR tokamak with Alfven wave heating. The Thomson scattering diagnostic is an upgraded version of the one previously installed at the ISTTOK tokamak, while the electron cyclotron emission radiometer employs a heterodyne sweeping radiometer. For purely Ohmic discharges, the electron temperature measurements from both diagnostics are in good agreement. Additional Alfven wave heating does not affect the capability of the Thomson scattering diagnostic to measure the instantaneous electron temperature, whereas measurements from the electron cyclotron emission radiometer become underestimates of the actual temperature values.
Elastic electron scattering from formic acid
Trevisan, Cynthia S.; Orel, Ann E.; Rescigno, Thomas N.
2006-07-31
Following our earlier study on the dynamics of low energy electron attachment to formic acid, we report the results of elastic low-energy electron collisions with formic acid. Momentum transfer and angular differential cross sections were obtained by performing fixed-nuclei calculations employing the complex Kohn variational method. We make a brief description of the technique used to account for the polar nature of this polyatomic target and compare our results with available experimental data.
Complete Solution of Electronic Excitation and Ionization in Electron-Hydrogen Molecule Scattering.
Zammit, Mark C; Savage, Jeremy S; Fursa, Dmitry V; Bray, Igor
2016-06-10
The convergent close-coupling method has been used to solve the electron-hydrogen molecule scattering problem in the fixed-nuclei approximation. Excellent agreement with experiment is found for the grand total, elastic, electronic-excitation, and total ionization cross sections from the very low to the very high energies. This shows that for the electronic degrees of freedom the method provides a complete treatment of electron scattering on molecules as it does for atoms. PMID:27341229
Complete solution of electronic excitation and ionization in electron-hydrogen molecule scattering
Zammit, Mark C.; Savage, Jeremy S.; Fursa, Dmitry V.; Bray, Igor
2016-06-01
The convergent close-coupling method has been used to solve the electron-hydrogen molecule scattering problem in the fixed-nuclei approximation. Excellent agreement with experiment is found for the grand total, elastic, electronic-excitation, and total ionization cross sections from the very low to the very high energies. This shows that for the electronic degrees of freedom the method provides a complete treatment of electron scattering on molecules as it does for atoms.
Complete Solution of Electronic Excitation and Ionization in Electron-Hydrogen Molecule Scattering
NASA Astrophysics Data System (ADS)
Zammit, Mark C.; Savage, Jeremy S.; Fursa, Dmitry V.; Bray, Igor
2016-06-01
The convergent close-coupling method has been used to solve the electron-hydrogen molecule scattering problem in the fixed-nuclei approximation. Excellent agreement with experiment is found for the grand total, elastic, electronic-excitation, and total ionization cross sections from the very low to the very high energies. This shows that for the electronic degrees of freedom the method provides a complete treatment of electron scattering on molecules as it does for atoms.
Energy distribution of elastically scattered electrons from double layer samples
NASA Astrophysics Data System (ADS)
Tőkési, K.; Varga, D.
2016-02-01
We present a theoretical description of the spectra of electrons elastically scattered from thin double layered Au-C samples. The analysis is based on the Monte Carlo simulation of the recoil and Doppler effects in reflection and transmission geometries of the scattering at a fixed angle of 44.3 ° and a primary energy of 40 keV. The relativistic correction is taken into account. Besides the experimentally measurable energy distributions the simulations give many partial distributions separately, depending on the number of elastic scatterings (single, and multiple scatterings of different types). Furthermore, we present detailed analytical calculations for the main parameters of the single scattering, taking into account both the ideal scattering geometry, i.e. infinitesimally small angular range, and the effect of the real, finite angular range used in the measurements. We show our results for intensity ratios, peak shifts and broadenings for four cases of measurement geometries and layer thicknesses. While in the peak intensity ratios of gold and carbon for transmission geometries were found to be in good agreement with the results of the single scattering model, especially large deviations were obtained in reflection geometries. The separation of the peaks, depending on the geometry and the thickness, generally smaller, and the peak width generally larger than it can be expected from the nominal values of the primary energy, scattering angle, and mean kinetic energy of the atoms. We also show that the peaks are asymmetric even for the case of the single scattering due to the finite solid angle. Finally, we present a qualitative comparison with the experimental data. We find our resulting energy distribution of elastically scattered electrons to be in good agreement with recent measurements.
Raman scattering in high-{Tc} superconductors: Electronic excitations
Cardona, M.; Strohm, T.; Kircher, J.
1996-12-31
Since the discovery of the high {Tc} superconductors Raman scattering has proven to be an excellent technique to characterize them and to investigate basic physical properties relevant to the elusive mechanism responsible for their superconductivity. The authors discuss here several aspects of the technique as applied to superconductivity, including scattering by lattice vibrations, magnetic excitations, and electronic excitations, with particular emphasis on the latter, both in the normal and the superconducting state. 47 refs., 8 figs., 1 tab.
Higher-order effects in inclusive electron-nucleus scattering.
Benhar, O.; Fabrocini, A.; Fantoni, S.; Pandharipande, V. R.; Pieper, S. C.; Sick, I.; Physics; INFIN; Univ. of Pisa; SISSA; Univ. of Illinois; SISSA; Univ. Basel
1995-10-05
Higher order corrections in the theory of inclusive scattering of high energy electrons by nuclear matter are studied. They involve at least three nucleons, and are due to: (i) the correlations among the spectator nucleons in matter, and (ii) the Pauli blocking of the scattering of the struck nucleon by a spectator nucleon. Their effect on the cross sections is found to be much smaller than those of the two-nucleon correlation hole and of color transparency.
Electron-impact scattering by arsine
NASA Astrophysics Data System (ADS)
Kaur, Jaspreet; Goswami, Biplab; Gupta, Dhanoj; Antony, Bobby
2014-07-01
We present elastic cross sections for electron interactions with arsine (AsH3) in gas phase over an extensive energy range from 0.5 to 5000 eV by combining two computational methods. The ab initio R-matrix method is employed for low-energy computations up to 15 eV and the intermediate to high-energy calculations were performed using the spherical complex optical potential (SCOP) method. The elastic cross section computed through the R matrix and SCOP formalism shows consistency at crossover energy (11-12 eV) and gives reasonable accord with the available data. Besides elastic cross sections, the differential cross section at low and intermediate incident electron energies is reported. The electronic excitation cross section is also reported at low energies. Shape resonance is observed at around 2.4 eV due to the formation of a transient negative ion state.
Low-energy scattering of electrons and positrons in liquids
NASA Technical Reports Server (NTRS)
Schrader, D. M.
1990-01-01
The scattering of low energy electrons and positrons is described for the liquid phase and compared and contrasted with that for the gas phase. Similarities as well as differences are noted. The loci of scattering sites, called spurs in the liquid phase, are considered in detail. In particular, their temporal and spatial evolution is considered from the point of view of scattering. Two emphases are made: one upon the stochastic calculation of the distribution of distances required for slowing down to thermal velocities, and the other upon the calculation of cross sections for energy loss by means of quantum mechanics.
Precision electroweak studies using parity violation in electron scattering
Paschke, K. D.
2013-11-07
The nature of new neutral-current interactions can be revealed at the low-energy precision frontier, where studies of parity-violation in electron scattering will complement the energy-frontier studies at the LHC. Measurements of the parity-violating observable A{sub PV} - the cross-section asymmetry in the scattering of longitudinally polarized electrons from an unpolarized target - are sensitive to possible contact interactions from new physics at multi-TeV mass scales. The 12 GeV upgrade at JLab and a new, high-intensity beam at Mainz offer opportunities for significant improvements in measurements of electron-electron and electron-quark parity-violating interactions.
Electron- and positron-proton elastic scattering in CLAS
L.B. Weinstein
2009-08-01
There is a significant disagreement between measurements of the proton electric form factor, G{sup p}{sub E}, using Rosenbluth separations and polarization transfer. This disagreement, if not explained, could pose a fundamental challenge to our understanding of electron scattering or proton structure. Two-photon exchange (TPE) processes, although not fully calculable, are the most likely explanation of this disagreement. We will definitively test this assertion by comparing the electron-proton and positron-proton elastic scattering cross section in the Jefferson Lab CLAS. We will make a mixed identical electron and positron tertiary beam by passing a 5.5 GeV primary electron beam through a radiator to make a photon beam and then passing the photon beam through a converter to make electron-positron pairs. Measuring the elastic cross sections simultaneously using identical lepton beams should significantly reduce systematic uncertainties.
Electron- and positron-proton elastic scattering in CLAS
Weinstein, L. B.
2009-09-02
There is a significant disagreement between measurements of the proton electric form factor, G{sup p}{sub E}, using Rosenbluth separations and polarization transfer. This disagreement, if not explained, could pose a fundamental challenge to our understanding of electron scattering or proton structure. Two-photon exchange (TPE) processes, although not fully calculable, are the most likely explanation of this disagreement. We will definitively test this assertion by comparing the electron-proton and positron-proton elastic scattering cross section in the Jefferson Lab CLAS. We will make a mixed identical electron and positron tertiary beam by passing a 5.5 GeV primary electron beam through a radiator to make a photon beam and then passing the photon beam through a converter to make electron-positron pairs. Measuring the elastic cross sections simultaneously using identical lepton beams should significantly reduce systematic uncertainties.
Hybrid Theory of Electron-Hydrogenic Systems Elastic Scattering
NASA Technical Reports Server (NTRS)
Bhatia, A. K.
2007-01-01
Accurate electron-hydrogen and electron-hydrogenic cross sections are required to interpret fusion experiments, laboratory plasma physics and properties of the solar and astrophysical plasmas. We have developed a method in which the short-range and long-range correlations can be included at the same time in the scattering equations. The phase shifts have rigorous lower bounds and the scattering lengths have rigorous upper bounds. The phase shifts in the resonance region can be used to calculate very accurately the resonance parameters.
Partial Wave Dispersion Relations: Application to Electron-Atom Scattering
NASA Technical Reports Server (NTRS)
Temkin, A.; Drachman, Richard J.
1999-01-01
In this Letter we propose the use of partial wave dispersion relations (DR's) as the way of solving the long-standing problem of correctly incorporating exchange in a valid DR for electron-atom scattering. In particular a method is given for effectively calculating the contribution of the discontinuity and/or poles of the partial wave amplitude which occur in the negative E plane. The method is successfully tested in three cases: (i) the analytically solvable exponential potential, (ii) the Hartree potential, and (iii) the S-wave exchange approximation for electron-hydrogen scattering.
Inelastic X-ray Scattering Studies of Electronic Excitations
NASA Astrophysics Data System (ADS)
Ishii, Kenji; Tohyama, Takami; Mizuki, Jun'ichiro
2013-02-01
Inelastic x-ray scattering (IXS) has developed into one of the most powerful momentum-resolved spectroscopies. Especially in the last decade, it has achieved significant progress utilizing brilliant x-rays from third-generation synchrotron radiation facilities. Simultaneously, theoretical efforts have been made to predict or interpret the experimental spectra. One of the scientific fields studied intensively by IXS is strongly correlated electron systems, where the interplay of charge, spin, and orbital degrees of freedom determines their physical properties. IXS can provide a new insight into the electron dynamics of the systems through the observation of charge, spin, and orbital excitations. Focusing on the momentum-resolved electronic excitations in strongly correlated electron systems, we review IXS studies and the present capabilities of IXS for the study of the dynamics of materials. With nonresonant inelastic x-ray scattering (NIXS), one can directly obtain dynamical charge correlation and we discuss its complementary aspects with inelastic neutron scattering. NIXS also has a unique capability of measuring higher multipole transitions, which are usually forbidden in conventional optical absorption. Resonant inelastic x-ray scattering (RIXS) is now established as a valuable tool for measuring charge, spin, and orbital excitations in a momentum-resolved manner. We describe RIXS works on cuprates in detail and show what kind of electronic excitations have been observed. We also discuss RIXS studies on other transition-metal compounds. Finally, we conclude with an outlook on IXS using next-generation x-ray sources.
Electron Scattering in Hot/Warm Plasmas
Rozsnyai, B F
2008-01-18
Electrical and thermal conductivities are presented for aluminum, iron and copper plasmas at various temperatures, and for gold between 15000 and 30000 Kelvin. The calculations are based on the continuum wave functions computed in the potential of the temperature and density dependent self-consistent 'average atom' (AA) model of the plasma. The cross sections are calculated by using the phase shifts of the continuum electron wave functions and also in the Born approximation. We show the combined effect of the thermal and radiative transport on the effective Rosseland mean opacities at temperatures from 1 to 1000 eV. Comparisons with low temperature experimental data are also presented.
Modeling Electron Pitch-Angle Scattering Rates by EMIC Waves
NASA Astrophysics Data System (ADS)
Usanova, Maria; Shprits, Yuri; Drozdov, Alexander
2016-07-01
The response of electron fluxes to different geomagnetic activity is determined by competing electron acceleration and loss processes. Interaction with EMIC waves is believed to be an important loss mechanism for the radiation belt electrons, which can undergo cyclotron resonance with EMIC waves and consequent pitch-angle scattering into the atmosphere. The recent study by Usanova et al. [2014] reported the first definitive proof of EMIC waves scattering electrons into the atmosphere. These new results are particularly interesting and significant as EMIC is the only wave mode that can scatter ultra-relativistic electrons much faster and more efficient than other wave modes (e.g., chorus and hiss) and therefore, is supposed to be a dominant internal loss mechanism for ˜>2 MeV energy electrons. In this talk we will focus on numerical modeling of EMIC-related electron losses. We compute bounce-averaged pitch-angle diffusion coefficients of electrons due to EMIC waves using a quasi-linear approach and use these coefficients as further input to the Versatile Electron Radiation Belt (VERB) diffusion code to simulate the evolution of electron phase space density during selected events. We will present a comparison of the simulation results and observed pitch angle distributions on the Van Allen Probes during selected events. We will also address the following questions: Where and under which conditions signatures of EMIC-related electron loss are typically observed? What are the EMIC wave and background plasma parameters required for this interaction? Can we reproduce observed losses of radiation belt electrons using numerical modeling?
Study of the (e,e'p) quasi-elastic reaction in complex nuclei: theory and experiment
Herraiz, Joaquin Lopez
2010-03-01
Experimental coincidence cross section and transverse-longitudinal asymmetry _{ATL} have been obtained for the quasielastic (e,e'p) reaction in ^{16}O, ^{12}C, and {sup 208}Pb in constant q-ω kinematics in the missing momentum range -350 < p_{miss} < 350 MeV/c. In these experiments, performed in experimental Hall A of the Thomas Jefferson National Accelerator Facility (JLAB), the beam energy and the momentum and angle of the scattered electrons were kept fixed, while the angle between the proton momentum and the momentum transfer q was varied in order to map out the missing momentum distribution. The experimental cross section and A_{TL} asymmetry have been compared with Monte Carlo simulations based on Distorted Wave Impulse Approximation (DWIA) calculations with both relativistic and non-relativistic spinor structure. The spectroscopic factors obtained for both models are in agreement with previous experimental values, while A_{TL} measurements favor the relativistic DWIA calculation. This thesis describes the details of the experimental setup, the calibration of the spectrometers, the techniques used in the data analysis to derive the final cross sections and the A_{TL}, the ingredients of the theoretical calculations employed and the comparison of the results with the simulations based on these theoretical models.
Elastic Scattering of Electron Vortex Beams in Magnetic Matter
NASA Astrophysics Data System (ADS)
Edström, Alexander; Lubk, Axel; Rusz, Ján
2016-03-01
Elastic scattering of electron vortex beams on magnetic materials leads to a weak magnetic contrast due to Zeeman interaction of orbital angular momentum of the beam with magnetic fields in the sample. The magnetic signal manifests itself as a redistribution of intensity in diffraction patterns due to a change of sign of the orbital angular momentum of the electron vortex beam. While in the atomic resolution regime the magnetic signal is most likely under the detection limits of present transmission electron microscopes, for electron probes with high orbital angular momenta, and correspondingly larger spatial extent, its detection is predicted to be feasible.
Controlling electron-phonon scattering with metamaterial plasmonic structures
NASA Astrophysics Data System (ADS)
Kempa, Krzysztof; Wu, Xueyuan; Kong, Jiantao; Broido, David
Electron-plasmon scattering can be faster than electron-phonon scattering. While in metals plasmons occur in the UV range, phonons dominate behavior at much lower frequencies (far IR range), and this typically decouples these phenomena. In metamaterial plasmonic structures, however, plasma effects can be tuned down to the far IR range, allowing for their interference with phonons. It was recently shown, that such interference can protect hot electron energy induced in a solar cell, from dissipation into heat. In this work we explore the possibility of using such an effect to control the electron-phonon interaction and transport in semiconductors. We demonstrate, that this could lead to a novel path to enhancing the electrical and thermal conductivities and the thermoelectric figure of merit.
Low-energy electron scattering by formic acid
Trevisan, C. S.; Orel, A. E.; Rescigno, T. N.
2006-10-15
We report the results of fixed-nuclei complex Kohn variational calculations of elastic electron scattering by formic acid, HCOOH. Momentum transfer and angular differential cross sections for incident electron energies ranging from 0.1 to 15 eV are presented and compared to available experimental data. The low-energy behavior of the cross section is analyzed and found to be consistent with the existence of a virtual state.
Applying a Trochoidal Electron Monochromator in Dissociative Electron Attachment Scattering
NASA Astrophysics Data System (ADS)
Arreola, Esmeralda
2016-03-01
Since the pioneering work of Boudiaffa et al., it has been understood that electrons, even with energies near or below the ionization threshold, are capable of initiating strand-breaks in human DNA. This discovery raised important questions for cancer treatments, since sub-ionizing electrons are known to be the most copiously produced secondary product of radiation therapy. But even to date these factors are largely excluded from dosimetry calculations. This lack of inclusion is, at least in part, certainly due to the dearth of fundamental data describing low-energy electron interactions with nucleotide molecules that form the basis of DNA. Understanding of how such slow electrons are able to damage DNA remains incomplete, but the strongly peaked nature of Boudiaffa et al.'s data gives strong hints at resonantly driven collision processes. DNA damage is therefore most likely driven by ``dissociative electron attachment'' (DEA). DEA is a rather complicated process to model due to the coupling of electronic and nuclear degrees of freedom in the molecule. At the California State University Fullerton, we are currently commissioning a new spectrometer to study dissociation channels, reaction rates and orientation effects in DEA collisions between slow electrons and nucleotide molecules. At the meeting we will present design parameters and commissioning data for this new apparatus.
Scaling in electron scattering from a relativistic Fermi gas
W. M. Alberico; A. Molinari; T. William Donnelly; E. L. Kronenberg; Wally Van Orden
1988-10-01
Within the context of the relativistic Fermi gas model, the concept of ''y scaling'' for inclusive electron scattering from nuclei is investigated. Specific kinematic shifts of the single-nucleon response in the nuclear medium can be incorporated with this model. Suggested generalizations beyond the strict Fermi gas model, including treatments of separated longitudinal and transverse responses, are also explored.
Modified effective range analysis of electron scattering from krypton
NASA Astrophysics Data System (ADS)
Fedus, Kamil
2014-10-01
The elastic cross sections for electron scattering on krypton from zero energy up to 10 eV have been analyzed by the modified effective range method. A simple model based on the analytical solution of the Schrödinger equation with the polarization potential using explicitly determined scattering phase shifts for the three lowest partial waves describes the elastic differential, integral and momentum transfer cross sections up to the energy threshold of the first inelastic process well. In detail, the contribution of the long-range polarization potential to the scattering phase shift is exactly expressed, while the contribution of the short-range effects is modelled by simple quadratic expressions (the effective range expansions). The effective range parameters are determined empirically by comparison with the latest experimental differential cross sections. Presently, the calculated integral and momentum transfer cross sections are validated against numerous electron scattering experiments and the most recent quantum-mechanical theories. To complete the picture, the two-term Boltzmann analysis is employed to determine the electron transport coefficients; the agreement with the electron swarm experimental data is found to be very good.
Examinations of electron temperature calculation methods in Thomson scattering diagnostics
Oh, Seungtae; Lee, Jong Ha; Wi, Hanmin
2012-10-15
Electron temperature from Thomson scattering diagnostic is derived through indirect calculation based on theoretical model. {chi}-square test is commonly used in the calculation, and the reliability of the calculation method highly depends on the noise level of input signals. In the simulations, noise effects of the {chi}-square test are examined and scale factor test is proposed as an alternative method.
Spin Structure Functions from Electron Scattering
Seonho Choi
2012-09-01
The spin structure of the nucleon can play a key testing ground for Quantum Chromo-Dynamics (QCD) at wide kinematic ranges from smaller to large four momentum transfer Q{sup 2}. The pioneering experiments have confirmed several QCD sum rules at high Q{sup 2} where a perturbative picture holds. For a full understanding of QCD at various scales, various measurements were made at intermediate and small Q{sup 2} region and their interpretation would be a challenging task due to the non-perturbative nature. Jefferson Lab has been one of the major experimental facilities for the spin structure with its polarized electron beams and various polarized targets. A few QCD sum rules have been compared with the measured spin structure functions g{sub 1}(x, Q{sup 2}) and g{sub 2}(x, Q{sup 2}) at low Q{sup 2} and surprising results have been obtained for the spin polarizabilities, {gamma}{sub 0} and {delta}{sub LT} . As for the proton spin structure functions, the lack of data for g{sub 2}(x,Q{sup 2}) structure functions has been complemented with a new experiment at Jefferson Lab, SANE. The results from SANE will provide a better picture of the proton spin structure at a wide kinematic range in x and Q{sup 2}.
Polarization of photons scattered by electrons in any spectral distribution
Chang, Zhe; Lin, Hai-Nan; Jiang, Yunguo
2014-01-01
On the basis of the quantum electrodynamics, we present a generic formalism of the polarization for beamed monochromatic photons scattered by electrons in any spectral distribution. The formulae reduce to the components of the Fano matrix when electrons are at rest. We mainly investigate the polarization in three scenarios, i.e., electrons at rest, isotropic electrons with a power-law spectrum, and thermal electrons. If the incident beam is polarized, the polarization is reduced significantly by isotropic electrons at large viewing angles; the degree of polarization caused by thermal electrons is about half of that caused by power-law electrons. If the incident bean is unpolarized, soft γ-rays can lead to about 15% polarization at viewing angles around π/4. For isotropic electrons, one remarkable feature is that the polarization as a function of the incident photon energy always peaks roughly at 1 MeV; this is valid for both the thermal and power-law cases. This feature can be used to distinguish the model of the inverse Compton scattering from that of the synchrotron radiation.
Electron scattering by magnetosonic waves in the inner magnetosphere
NASA Astrophysics Data System (ADS)
Ma, Qianli; Li, Wen; Thorne, Richard M.; Bortnik, Jacob; Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.
2016-01-01
We investigate the importance of electron scattering by magnetosonic waves in the Earth's inner magnetosphere. A statistical survey of the magnetosonic wave amplitude and wave frequency spectrum, as a function of geomagnetic activity, is performed using the Van Allen Probes wave measurements and is found to be generally consistent with the wave distribution obtained from previous spacecraft missions. Outside the plasmapause the statistical frequency distribution of magnetosonic waves follows the variation of the lower hybrid resonance frequency, but this trend is not observed inside the plasmasphere. Drift and bounce averaged electron diffusion rates due to magnetosonic waves are calculated using a recently developed analytical formula. The resulting timescale of electron energization during disturbed conditions (when AE* > 300 nT) is more than 10 days. We perform a 2-D simulation of the electron phase space density evolution due to magnetosonic wave scattering during disturbed conditions. Outside the plasmapause, the waves accelerate electrons with pitch angles between 50° and 70° and form butterfly pitch angle distributions at energies from ~100 keV to a few MeV over a timescale of several days; whereas inside the plasmapause, the electron acceleration is very weak. Our study suggests that intense magnetosonic waves may cause the butterfly distribution of radiation belt electrons especially outside the plasmapause, but electron acceleration due to magnetosonic waves is generally not as effective as chorus wave acceleration.
Predicting reaction observables from back-scattering measurements in low-energy heavy-ion collisions
NASA Astrophysics Data System (ADS)
Diaz-Torres, A.; Sargsyan, V. V.; Adamian, G. G.; Antonenko, N. V.; Gomes, P. R. S.; Lenske, H.
2016-01-01
A simplified, reliable and useful method, based on reaction theory, for calculating a number of integrated and differential cross sections in low-energy heavy-ion collisions is presented. Simplified formulae provide predictions of reaction, capture and elastic-scattering differential cross sections, using experimental information about elastic and quasi-elastic back-scattering excitation functions.
Precise polarization measurements via detection of compton scattered electrons
Tvaskis, Vladas; Dutta, Dipangkar; Gaskell, David J.; Narayan, Amrendra
2014-01-01
The Qweak experiment at Jefferson Lab aims to make a 4% measurement of the parity-violating asymmetry in elastic scattering at very low Q{sup 2} of a longitudinally polarized electron beam off a proton target. One of the dominant experimental systematic uncertainties in Qweak will result from determining the beam polarization. A new Compton polarimeter was installed in the fall of 2010 to provide a non-invasive and continuous monitoring of the electron beam polarization in Hall C at Jefferson Lab. The Compton-scattered electrons are detected in four planes of diamond micro-strip detectors. We have achieved the design goals of <1% statistical uncertainty per hour and expect to achieve <1% systematic uncertainty.
Goeppert-Mayer Award Recipient: Electron Scattering and Nucleon Structure
NASA Astrophysics Data System (ADS)
Beise, Elizabeth
1998-04-01
Electron scattering from hydrogen and light nuclear targets has long been recognized as one of the best tools for understanding the electromagnetic structure of protons, neutrons and few-nucleon systems. In the last decade, considerable progress has been made in the field through advances in polarized beams and polarized targets. Improvements in polarized electron sources has made it feasible to also study the structure of the nucleon through parity-violating electron scattering, where the nucleon's neutral weak structure is probed. In this talk, a summary of the present experimental status of the nucleon's electroweak structure will be presented, with an emphasis on recent results from the MIT-Bates and Jefferson Laboratories.
Parity Violation in Forward Angle Elastic Electron-Proton Scattering
Miller, IV, Grady Wilson
2001-01-01
We have measured the parity-violating electroweak asymmetry in the elastic scattering of polarized electrons from the proton at Jefferson Laboratory. The kinematic point ({theta}_lab = 12.3 deg. and (Q^2) = 0.48 (GeV/c)^2) is chosen to provide sensitivity to the strange electric form factor G^s_E. A 3.36 GeV beam of longitudinally polarized electrons was scattered from protons in a liquid hydrogen target. The scattered flux was detected by a pair of spectrometers which focussed the elastically-scattered electrons onto total-absorption detectors. The detector signals were integrated and digitized by a custom data acquisition system. A feedback system reduced systematic errors by controlling helicity-correlated beam intensity differences at the sub-ppm (part per million) level. The experimental result, A = 14.5 +/- 2.0 (stat) +/- 1.1 (syst) ppm, is consistent with the electroweak Standard Model with no additional contributions from strange quarks. In particular, the measurement implies G^S_E + 0.39 G^s_M = 0.023 +/- 0.040 +/- 0.026 ({delta}G^n_E), where the last uncertainty is due to the estimated uncertainty in the neutron electric form factor G^n_E . This result represents the first experimental constraint of the strange electric form factor.
Nonlinear single Compton scattering of an electron wave packet
NASA Astrophysics Data System (ADS)
Angioi, A.; Mackenroth, F.; Di Piazza, A.
2016-05-01
Nonlinear single Compton scattering has been thoroughly investigated in the literature under the assumption that the electron initially has a definite momentum. Here, we study a more general initial state and consider the electron as a wave packet. In particular, we investigate the energy spectrum of the emitted radiation and show that, in typical experimental situations, some features of the spectra shown in previous works are almost completely washed out. Moreover, we show that, at comparable relative uncertainties, the one in the momentum of the incoming electron has a larger impact on the photon spectra at a fixed observation direction than the one on the laser frequency.
Cross sections for electron scattering from α-tetrahydrofurfuryl alcohol
NASA Astrophysics Data System (ADS)
Duque, H. V.; Chiari, L.; Jones, D. B.; Thorn, P. A.; Pettifer, Z.; da Silva, G. B.; Limão-Vieira, P.; Duflot, D.; Hubin-Franskin, M.-J.; Delwiche, J.; Blanco, F.; García, G.; Lopes, M. C. A.; Ratnavelu, K.; White, R. D.; Brunger, M. J.
2014-07-01
We report on measurements of integral cross sections (ICSs) for electron impact excitation of a series of Rydberg electronic-states in α-tetrahydrofurfuryl alcohol. The energy range of these experiments was 20-50 eV. There are currently no other results against which we can directly compare those measured data. We also report results from our independent atom model with screened additivity rule correction computations, namely for the total cross section, elastic ICS, inelastic ICS (all discrete electronic states and neutral dissociation) and the total ionisation ICS. Where possible, our calculated cross sections are compared to the limited available data of each scattering process.
Anion Photoelectron Angular Distributions: Electron Scattering Resonances in Photodetachment
NASA Astrophysics Data System (ADS)
Mabbs, Richard
2012-06-01
To a large degree the photoelectron angular distributions (PAD) of anionic species represent signatures of the bound parent orbital. However, these angular distributions are also influenced by interaction of the outgoing electron with the neutral (atomic, molecular or cluster) residue. The electron kinetic energy evolution (eKE) of the PAD is presented for a number of different species (from molecular to cluster anion), showing the often striking effect of excitation of temporary excited anionic states. These cases highlight the influence of different types of electron-molecule scattering resonances in photodetachment dynamics. Additionally, the possibility of using the eKE evolution of the PAD for structural elucidation is discussed.
APD detector electronics for the NSTX Thomson scattering system
D.W. Johnson; B.P. LeBlanc; D.L. Long; G. Renda
2000-08-07
An electronics system has been installed and tested for the readout of APD detectors for the NSTX Thomson scattering system. Similar to previous designs, it features preamps with a fast and a slow output. The fast output uses pulse shaping to optimize sensitivity for the 8 nsec scattered light pulse while rejecting noise in the intrinsic plasma background. A low readout noise of {approximately}25 photoelectrons is achieved at an APD gain of 75. The design incorporates a number of features to provide flexibility for various modes of calibration.
Resonance electronic Raman scattering in rare earth crystals
Williams, G.M.
1988-11-10
The intensities of Raman scattering transitions between electronic energy levels of trivalent rare earth ions doped into transparent crystals were measured and compared to theory. A particle emphasis was placed on the examination of the effect of intermediate state resonances on the Raman scattering intensities. Two specific systems were studied: Ce/sup 3 +/(4f/sup 1/) in single crystals of LuPO/sub 4/ and Er/sup 3 +/(4f/sup 11/) in single crystals of ErPO/sub 4/. 134 refs., 92 figs., 33 tabs.
Electron scattering by laser-excited barium atoms
NASA Technical Reports Server (NTRS)
Register, D. F.; Trajmar, S.; Jensen, S. W.; Poe, R. T.
1978-01-01
Inelastic and superelastic scattering of 30- and 100-eV electrons by laser-excited 6s 6p 1P and subsequent cascade-populated 6s 6p 3P, 6s 5d 1D, and 6s 5d 3D Ba atoms have been observed. Absolute differential cross sections for the singlet and relative scattering intensities for the triplet species have been determined in the 5 to 20 deg angular region. Under the present conditions excitations dominate over deexcitations.
Technology Transfer Automated Retrieval System (TEKTRAN)
The need to increase the use of low valued co-products derived from the processing of sugar beets has prompted the investigation of the structure of the pectin extracted from sugar beet pulp. The characterization of sugar beet pectin is essential as it has the potential to be used in the production ...
Theoretical Study of Electron Scattering By Small Clusters and Adsorbates
NASA Technical Reports Server (NTRS)
Huo, Winifred M.; Sheehy, J. A.
1994-01-01
Current interest in clusters stems from their role as novel materials as well as a possible extension of cluster results to bulk systems. Experimental investigations on clusters have been carried out using laser spectroscopy, microwave spectroscopy, heavy-particle collisions, as well as electron collisions with earlier experimental work on electron attachment and ionization having been reviewed previously. Recently, Mark and coworkers studied the decay channels of cluster ions following electron impact ionization. Rauth et al. reported the formation of the superhalogen ion SF7(-) and other nonstoichiometric cluster ions in their study of electron attachment to SF6 clusters. Kresin et al. measured the absolute electron-impact depletion cross section of metal clusters Na8, Na(20), and Na(40). They found that the inelastic scattering cross section increased with cluster size and was considerably greater than the hard sphere collision cross sections. They hypothesized that electron attachment and collision-induced fragmentation were the dominant physical processes responsible for this effect. For the two smaller clusters, they also found a sharp increase in the cross section near threshold. Most theoretical studies of clusters have been devoted to their electronic structures, vibrational relaxation, and predissociation while investigations of electron scattering from clusters has been lacking. In view of this, we recently undertook an ab initio study of electron scattering from small Be clusters and BeCO. Beryllium was chosen because it is readily amenable to ab t'nitio calculations. Moreover, the electronic structure of Be clusters has been studied extensively, showing that the Be-Be bond is relatively weak in comparison with a normal chemical bond. Our investigation focuses on how the cross sections change with cluster size and geometry. The range of energy studied, 0.05 - 5.0 eV, is chosen because of the ubiquitous resonance in the low-energy scattering of Be. Hence
Kinetic Enhancement of Raman Backscatter, and Electron Acoustic Thomson Scatter
Strozzi, D J; Williams, E A; Langdon, A B; Bers, A
2006-09-01
1-D Eulerian Vlasov-Maxwell simulations are presented which show kinetic enhancement of stimulated Raman backscatter (SRBS) due to electron trapping in regimes of heavy linear Landau damping. The conventional Raman Langmuir wave is transformed into a set of beam acoustic modes [L. Yin et al., Phys. Rev. E 73, 025401 (2006)]. For the first time, a low phase velocity electron acoustic wave (EAW) is seen developing from the self-consistent Raman physics. Backscatter of the pump laser off the EAW fluctuations is reported and referred to as electron acoustic Thomson scatter. This light is similar in wavelength to, although much lower in amplitude than, the reflected light between the pump and SRBS wavelengths observed in single hot spot experiments, and previously interpreted as stimulated electron acoustic scatter [D. S. Montgomery et al., Phys. Rev. Lett. 87, 155001 (2001)]. The EAW observed in our simulations is strongest well below the phase-matched frequency for electron acoustic scatter, and therefore the EAW is not produced by it. The beating of different beam acoustic modes is proposed as the EAW excitation mechanism, and is called beam acoustic decay. Supporting evidence for this process, including bispectral analysis, is presented. The linear electrostatic modes, found by projecting the numerical distribution function onto a Gauss-Hermite basis, include beam acoustic modes (some of which are unstable even without parametric coupling to light waves) and a strongly-damped EAW similar to the observed one. This linear EAW results from non-Maxwellian features in the electron distribution, rather than nonlinearity due to electron trapping.
Modeling dynamical electron scattering with Bethe potentials and the scattering matrix.
Wang, A; De Graef, M
2016-01-01
Bethe potentials were introduced by Bethe in 1928 as a first order perturbation approach to reducing the number of diffracted beams in dynamical electron scattering problems. The approach starts from the Bloch wave representation, and uses a threshold criterion to split the diffracted beams into two subsets, namely strong and weak beams. Since the use of Bloch wave based Bethe potentials for defect simulations is somewhat tedious, this paper applies the perturbation approach to the scattering matrix formalism, which is more readily adaptable for defect image simulations. The size of the dynamical matrix, and hence the computation time, can be reduced significantly. A threshold criterion for the separation of scattered beams into strong and weak sets is introduced. A general guideline in setting the threshold for strong or weak beam selection is discussed along with several parameters that may influence the threshold values, such as atomic number, accelerating voltage, structure complexity, incident beam tilt and temperature. PMID:26433091
J.C. Cornejo, J.L. Herraiz, A. Camsonne, A. Saha, J.M. Udias, G. Urciuoli, J.R. Vignote, K.A. Aniol
2012-09-01
Quasi elastic cross sections were measured for the first time for both negative and positive missing momenta for the {sup 209}Bi(e,e'p){sup 208}Pb reaction leading to the ground state and hole states of (208)Pb. Experimental cross sections obtained between -0.3 GeV/c to 0.3 GeV/c agree with theoretical calculations using RDWIA techniques both in shape and magnitude for the ground state. The data for the ground state production of {sup 208}Pb are consistent with a theoretical model assuming a single proton(1.06 +- 0.10) in the 1h9/2 orbit in {sup 209}Bi.
Elastic scattering of electrons from singly ionized argon
Griffin, D.C.; Pindzola, M.S.
1996-03-01
Recently, Greenwood {ital et} {ital al}. [Phys. Rev. Lett. {bold 75}, 1062 (1995)] reported measurements of large-angle elastic scattering of electrons from singly ionized argon at an energy of 3.3 eV. They compared their results for the differential cross section with cross sections determined using phase shifts obtained from two different scattering potentials and found large discrepancies between theory and experiment at large angles. They state that these differences may be due to the effects of polarization of the target, which are not included in their calculations, as well as inaccurate representations of electron exchange in the local scattering potentials that are employed to determine the phase shifts. In order to test these proposed explanations of the discrepancies, we have carried out calculations of elastic scattering from Ar{sup +} using the {ital R}-matrix method. We compare both a single-state calculation, which does not include polarization, and a 17-state calculation, in which the effects of dipole polarizability are included through the use of polarization pseudostates within the close-coupling expansion, to each other and with the measurements. We find some differences between the two calculations at intermediate scattering angles, but very close agreement at angles above 100{degree}. Although the calculated cross sections agree with experiment between 120{degree} and 135{degree}, large discrepancies persist at angles above 135{degree}. We conclude that the differences between the measurements and theory cannot be explained on the basis of an inaccurate representation of electron exchange or polarization of the target. {copyright} {ital 1996 The American Physical Society.}
Generalized Hartree-Fock method for electron-atom scattering
Rosenberg, L.
1997-09-01
In the widely used Hartree-Fock procedure for atomic structure calculations, trial functions in the form of linear combinations of Slater determinants are constructed and the Rayleigh-Ritz minimum principle is applied to determine the best in that class. A generalization of this approach, applicable to low-energy electron-atom scattering, is developed here. The method is based on a unique decomposition of the scattering wave function into open- and closed-channel components, so chosen that an approximation to the closed-channel component may be obtained by adopting it as a trial function in a minimum principle, whose rigor can be maintained even when the target wave functions are imprecisely known. Given a closed-channel trial function, the full scattering function may be determined from the solution of an effective one-body Schr{umlt o}dinger equation. Alternatively, in a generalized Hartree-Fock approach, the minimum principle leads to coupled integrodifferential equations to be satisfied by the basis functions appearing in a Slater-determinant representation of the closed-channel wave function; it also provides a procedure for optimizing the choice of nonlinear parameters in a variational determination of these basis functions. Inclusion of additional Slater determinants in the closed-channel trial function allows for systematic improvement of that function, as well as the calculated scattering parameters, with the possibility of spurious singularities avoided. Electron-electron correlations can be important in accounting for long-range forces and resonances. These correlation effects can be included explicitly by suitable choice of one component of the closed-channel wave function; the remaining component may then be determined by the generalized Hartree-Fock procedure. As a simple test, the method is applied to s-wave scattering of positrons by hydrogen. {copyright} {ital 1997} {ital The American Physical Society}
Low-energy positron and electron scattering from nitrogen dioxide
NASA Astrophysics Data System (ADS)
Chiari, Luca; Zecca, Antonio; García, Gustavo; Blanco, Francisco; Brunger, M. J.
2013-12-01
Total cross section (TCS) measurements for positron scattering from nitrogen dioxide (NO2) are presented in the energy range 0.2-40 eV. The TCS, the elastic integral and differential cross sections, and the integral cross section accounting of all the inelastic processes (including positronium formation) have also been computed using the independent atom model with screening corrected additivity rule (IAM-SCAR) for incident energies from 1 to 1000 eV. A qualitative level of agreement is found between the present TCS experiment and theory at the common energies. As no previous measurements or calculations for positron-NO2 scattering exist in the literature, we also computed the TCS for electron collisions with NO2 employing the IAM-SCAR method. A comparison of those results to the present positron cross sections and the earlier electron-impact data and calculations is provided. To investigate the role that chemical substitution plays in positron scattering phenomena, we also compare the present positron-NO2 data with the TCSs measured at the University of Trento for positron scattering from N2O and CO2.
Influence of the nuclear medium on inclusive electron and neutrino scattering off nuclei
Buss, O.; Leitner, T.; Mosel, U.; Alvarez-Ruso, L.
2007-09-15
We present a model for inclusive electron and neutrino scattering off nuclei paying special attention to the influence of in-medium effects on the quasielastic scattering and pion-production mechanisms. Our results for electron scattering off {sup 16}O are compared to experimental data at beam energies ranging from 0.7 to 1.5 GeV. The good description of electron scattering serves as a benchmark for neutrino scattering.
Calculation of electron scattering from the ground state of ytterbium
Bostock, Christopher J.; Fursa, Dmitry V.; Bray, Igor
2011-05-15
We report on the application of the convergent close-coupling method, in both relativistic and nonrelativistic formulations, to electron scattering from ytterbium. Angle-differential and integrated cross sections are presented for elastic scattering and excitation of the states (6s6p){sup 3}P{sub 0,1,2}, (6s6p){sup 1}P{sub 1}{sup o}, (6s7p){sup 1}P{sub 1}{sup o}, and (6s5d){sup 1}D{sub 2}{sup e} for a range of incident electron energies. We also present calculations of the total cross section, and angle-differential Stokes parameters for excitation of the (6s6p){sup 3}P{sub 1}{sup o} state from the ground state. A comparison is made with the relativistic distorted-wave method and experiments.
Multiple electronic Raman scatterings in a single metallic carbon nanotube
NASA Astrophysics Data System (ADS)
Zhang, Daqi; Yang, Juan; Hasdeo, Eddwi H.; Liu, Can; Liu, Kaihui; Saito, Riichiro; Li, Yan
2016-06-01
We observe multiple electronic Raman scatterings (ERSs) in a single suspended metallic single-walled carbon nanotube. The ERS process originates from the inelastic scattering of photoexcited excitons by a continuum of low-lying electron-hole pairs. In previous work, the observed Fano factor of the G band line shape is always negative; however, in this work we find that the Fano factor can be either positive or negative depending on the relative position of the nearest ERS with respect to the G band. This supports the idea that the origin of the G band asymmetry is an interference between the discrete G band and the continuous ERS. We also report that the ERS position and intensity are sensitive to the nanotube bundling effect and the laser heating effect.
Theory of high-energy electron scattering by composite targets
Coester, F.
1988-01-01
The emphasis of these expository lectures is on the role of relativistic invariance and the unity of the theory for medium and high energies. Sec. 2 introduces the kinematic notation and provides an elementary derivation of the general cross section. The relevant properties of the Poincare group and the transformation properties of current operators and target states are described in Sec 3. In Sec. 4 representations of target states with kinematic light-front symmetry are briefly discussed. The focus is on two applications. An impulse approximation of inclusive electron nucleus scattering at both medium and high energies. A parton model of the proton applied to deep inelastic scattering of polarized electrons by polarized protons. 19 refs.
Elastic Electron Scattering from Tritium and Helium-3
DOE R&D Accomplishments Database
Collard, H.; Hofstadter, R.; Hughes, E. B.; Johansson, A.; Yearian, M. R.; Day, R. B.; Wagner, R. T.
1964-10-01
The mirror nuclei of tritium and helium-3 have been studied by the method of elastic electron scattering. Absolute cross sections have been measured for incident electron energies in the range 110 - 690 MeV at scattering angles lying between 40 degrees and 135 degrees in this energy range. The data have been interpreted in a straightforward manner and form factors are given for the distributions of charge and magnetic moment in the two nuclei over a range of four-momentum transfer squared 1.0 - 8.0 F{sup -2}. Model-independent radii of the charge and magnetic moment distributions are given and an attempt is made to deduce form factors describing the spatial distribution of the protons in tritium and helium-3.
Measurement of neutrino flux from neutrino-electron elastic scattering
Park, J.; Aliaga, L.; Altinok, O.; Bellantoni, L.; Bercellie, A.; Betancourt, M.; Bodek, A.; Bravar, A.; Budd, H.; Cai, T.; et al
2016-06-10
In muon-neutrino elastic scattering on electrons is an observable neutrino process whose cross section is precisely known. Consequently a measurement of this process in an accelerator-based νμ beam can improve the knowledge of the absolute neutrino flux impinging upon the detector; typically this knowledge is limited to ~10% due to uncertainties in hadron production and focusing. We also isolated a sample of 135±17 neutrino-electron elastic scattering candidates in the segmented scintillator detector of MINERvA, after subtracting backgrounds and correcting for efficiency. We show how this sample can be used to reduce the total uncertainty on the NuMI νμ flux frommore » 9% to 6%. Finally, our measurement provides a flux constraint that is useful to other experiments using the NuMI beam, and this technique is applicable to future neutrino beams operating at multi-GeV energies.« less
Measurement of neutrino flux from neutrino-electron elastic scattering
NASA Astrophysics Data System (ADS)
Park, J.; Aliaga, L.; Altinok, O.; Bellantoni, L.; Bercellie, A.; Betancourt, M.; Bodek, A.; Bravar, A.; Budd, H.; Cai, T.; Carneiro, M. F.; Christy, M. E.; Chvojka, J.; da Motta, H.; Dytman, S. A.; Díaz, G. A.; Eberly, B.; Felix, J.; Fields, L.; Fine, R.; Gago, A. M.; Galindo, R.; Ghosh, A.; Golan, T.; Gran, R.; Harris, D. A.; Higuera, A.; Kleykamp, J.; Kordosky, M.; Le, T.; Maher, E.; Manly, S.; Mann, W. A.; Marshall, C. M.; Martinez Caicedo, D. A.; McFarland, K. S.; McGivern, C. L.; McGowan, A. M.; Messerly, B.; Miller, J.; Mislivec, A.; Morfín, J. G.; Mousseau, J.; Naples, D.; Nelson, J. K.; Norrick, A.; Nuruzzaman; Osta, J.; Paolone, V.; Patrick, C. E.; Perdue, G. N.; Rakotondravohitra, L.; Ramirez, M. A.; Ray, H.; Ren, L.; Rimal, D.; Rodrigues, P. A.; Ruterbories, D.; Schellman, H.; Solano Salinas, C. J.; Tagg, N.; Tice, B. G.; Valencia, E.; Walton, T.; Wolcott, J.; Wospakrik, M.; Zavala, G.; Zhang, D.; Miner ν A Collaboration
2016-06-01
Muon-neutrino elastic scattering on electrons is an observable neutrino process whose cross section is precisely known. Consequently a measurement of this process in an accelerator-based νμ beam can improve the knowledge of the absolute neutrino flux impinging upon the detector; typically this knowledge is limited to ˜10 % due to uncertainties in hadron production and focusing. We have isolated a sample of 135 ±17 neutrino-electron elastic scattering candidates in the segmented scintillator detector of MINERvA, after subtracting backgrounds and correcting for efficiency. We show how this sample can be used to reduce the total uncertainty on the NuMI νμ flux from 9% to 6%. Our measurement provides a flux constraint that is useful to other experiments using the NuMI beam, and this technique is applicable to future neutrino beams operating at multi-GeV energies.
Quasielastic electron-deuteron scattering in the weak binding approximation
Ethier, Jacob J.; Doshi, Nidhi P.; Malace, Simona P.; Melnitchouk, Wally
2014-06-01
We perform a global analysis of all available electron-deuteron quasielastic scattering data using Q^2-dependent smearing functions that describe inclusive inelastic e-d scattering within the weak binding approximation. We study the dependence of the cross sections on the deuteron wave function and the off-shell extrapolation of the elastic electron-nucleon cross section, which show particular sensitivity at x >> 1. The excellent overall agreement with data over a large range of Q^2 and x suggest a limited need for effects beyond the impulse approximation, with the exception of the very high-x or very low-Q^2 regions, where short-distance effects in the deuteron become more relevant.
Electron Scattering at Surfaces and Interfaces of Transition Metals
NASA Astrophysics Data System (ADS)
Zheng, Pengyuan
The effect of surfaces on the electron transport at reduced scales is attracting continuous interest due to its broad impact on both the understanding of materials properties and their application for nanoelectronics. The size dependence of for conductor's electrical resistivity rho due to electron surface scattering is most commonly described within the framework of Fuchs and Sondheimer (FS) and their various extensions, which uses a phenomenological scattering parameter p to define the probability of electrons being elastically (i.e. specularly) scattered by the surface without causing an increase of rho at reduced size. However, a basic understanding of what surface chemistry and structure parameters determine the specularity p is still lacking. In addition, the assumption of a spherical Fermi surface in the FS model is too simple for transition metals to give accurate account of the actual surface scattering effect. The goal of this study is to develop an understanding of the physics governing electron surface/interface scattering in transition metals and to study the significance of their Fermi surface shape on surface scattering. The advancement of the scientific knowledge in electron surface and interface scattering of transition metals can provide insights into how to design high-conductivity nanowires that will facilitate the viable development of advanced integrated circuits, thermoelectric power generation and spintronics. Sequential in situ and ex situ transport measurements as a function of surface chemistry demonstrate that electron surface/interface scattering can be engineered by surface doping, causing a decrease in the rho. For instance, the rho of 9.3-nm-thick epitaxial and polycrystalline Cu is reduced by 11--13% when coated with 0.75 nm Ni. This is due to electron surface scattering which exhibits a specularity p = 0.7 for the Cu-vacuum interface that transitions to completely diffuse (p = 0) when exposed to air. In contrast, Ni-coated surfaces
Short Range Correlations, Inclusive Electron-Nucleus Scattering, and Scaling
Day, Donal
2008-10-13
The presence of high momentum components in the nuclear wavefunction has been of great interest for many years. Unfortunately high momentum components, associated with the short range correlations (SRC), have been difficult to isolate unambiquously. Inclusive electron scattering cross sections in the quasielastic region have been measured over a wide range of energy and momentum transfers from very light to very heavy nuclei and the scaling analyses of these data can provide useful information on the presence of SRCs and more.
Electron scattering in graphene with adsorbed NaCl nanoparticles
Drabińska, Aneta Kaźmierczak, Piotr; Bożek, Rafał; Karpierz, Ewelina; Wysmołek, Andrzej; Kamińska, Maria; Wołoś, Agnieszka; Krajewska, Aleksandra
2015-01-07
In this work, the results of contactless magnetoconductance and Raman spectroscopy measurements performed for a graphene sample after its immersion in NaCl solution were presented. The properties of the immersed sample were compared with those of a non-immersed reference sample. Atomic force microscopy and electron spin resonance experiments confirmed the deposition of NaCl nanoparticles on the graphene surface. A weak localization signal observed using contactless magnetoconductance showed the reduction of the coherence length after NaCl treatment of graphene. Temperature dependence of the coherence length indicated a change from ballistic to diffusive regime in electron transport after NaCl treatment. The main inelastic scattering process was of the electron-electron type but the major reason for the reduction of the coherence length at low temperatures was additional, temperature independent, inelastic scattering. We associate it with spin flip scattering, caused by NaCl nanoparticles present on the graphene surface. Raman spectroscopy showed an increase in the D and D′ bands intensities for graphene after its immersion in NaCl solution. An analysis of the D, D′, and G bands intensities proved that this additional scattering is related to the decoration of vacancies and grain boundaries with NaCl nanoparticles, as well as generation of new on-site defects as a result of the decoration of the graphene surface with NaCl nanoparticles. The observed energy shifts of 2D and G bands indicated that NaCl deposition on the graphene surface did not change carrier concentration, but reduced compressive biaxial strain in the graphene layer.
Two-photon exchange and elastic electron-proton scattering
Peter Blunden; Wally Melnitchouk; John Tjon
2003-06-01
Two-photon exchange contributions to elastic electron-proton scattering cross sections are evaluated in a simple hadronic model including the finite size of the proton. The corrections are found to be small, but with a strong angular dependence at fixed Q{sup 2}. This is significant for the Rosenbluth technique for determining the ratio of electric and magnetic form factors of the proton, and partly reconciles the apparent discrepancy with the results of the polarization transfer technique.
NASA Astrophysics Data System (ADS)
Fu, H.; Scales, W. A.; Bernhardt, P. A.; Samimi, A.; Mahmoudian, A.; Briczinski, S. J.; McCarrick, M. J.
2013-09-01
Results of secondary radiation, Stimulated Electromagnetic Emission (SEE), produced during ionospheric modification experiments using ground-based high-power radio waves are reported. These results obtained at the High Frequency Active Auroral Research Program (HAARP) facility specifically considered the generation of Magnetized Stimulated Brillouin Scatter (MSBS) and Stimulated Ion Bernstein Scatter (SIBS) lines in the SEE spectrum when the transmitter frequency is near harmonics of the electron gyrofrequency. The heater antenna beam angle effect was investigated on MSBS in detail and shows a new spectral line postulated to be generated near the upper hybrid resonance region due to ion acoustic wave interaction. Frequency sweeping experiments near the electron gyroharmonics show for the first time the transition from MSBS to SIBS lines as the heater pump frequency approaches the gyroharmonic. Significantly far from the gyroharmonic, MSBS lines dominate, while close to the gyroharmonic, SIBS lines strengthen while MSBS lines weaken. New possibilities for diagnostic information are discussed in light of these new observations.
Dual scattering foil design for poly-energetic electron beams.
Kainz, K K; Antolak, J A; Almond, P R; Bloch, C D; Hogstrom, K R
2005-03-01
The laser wakefield acceleration (LWFA) mechanism can accelerate electrons to energies within the 6-20 MeV range desired for therapy application. However, the energy spectrum of LWFA-generated electrons is broad, on the order of tens of MeV. Using existing laser technology, the therapeutic beam might require a significant energy spread to achieve clinically acceptable dose rates. The purpose of this work was to test the assumption that a scattering foil system designed for a mono-energetic beam would be suitable for a poly-energetic beam with a significant energy spread. Dual scattering foil systems were designed for mono-energetic beams using an existing analytical formalism based on Gaussian multiple-Coulomb scattering theory. The design criterion was to create a flat beam that would be suitable for fields up to 25 x 25 cm2 at 100 cm from the primary scattering foil. Radial planar fluence profiles for poly-energetic beams with energy spreads ranging from 0.5 MeV to 6.5 MeV were calculated using two methods: (a) analytically by summing beam profiles for a range of mono-energetic beams through the scattering foil system, and (b) by Monte Carlo using the EGS/BEAM code. The analytic calculations facilitated fine adjustments to the foil design, and the Monte Carlo calculations enabled us to verify the results of the analytic calculation and to determine the phase-space characteristics of the broadened beam. Results showed that the flatness of the scattered beam is fairly insensitive to the width of the input energy spectrum. Also, results showed that dose calculated by the analytical and Monte Carlo methods agreed very well in the central portion of the beam. Outside the useable field area, the differences between the analytical and Monte Carlo results were small but significant, possibly due to the small angle approximation. However, these did not affect the conclusion that a scattering foil system designed for a mono-energetic beam will be suitable for a poly
Landau retardation on the occurrence scattering time in quantum electron-hole plasmas
NASA Astrophysics Data System (ADS)
Hong, Woo-Pyo; Jung, Young-Dae
2016-03-01
The Landau damping effects on the occurrence scattering time in electron collisions are investigated in a quantum plasma composed of electrons and holes. The Shukla-Stenflo-Bingham effective potential model is employed to obtain the occurrence scattering time in a quantum electron-hole plasma. The result shows that the influence of Landau damping produces the imaginary term in the scattering amplitude. It is then found that the Landau damping generates the retardation effect on the occurrence scattering time. It is found that the occurrence scattering time increases in forward scattering domains and decreases in backward scattering domains with an increase of the Landau parameter. It is also found that the occurrence scattering time decreases with increasing collision energy. In addition, it is found that the quantum shielding effect enhances the occurrence scattering time in the forward scattering and, however, suppresses the occurrence scattering time in the backward scattering.
Low-Energy Elastic Electron Scattering by Atomic Oxygen
NASA Technical Reports Server (NTRS)
Zatsarinny O.; Bartschat, K.; Tayal, S. S.
2006-01-01
The B-spline R-matrix method is employed to investigate the low-energy elastic electron scattering by atomic oxygen. Flexible non-orthogonal sets of radial functions are used to construct the target description and to represent the scattering functions. A detailed investigation regarding the dependence of the predicted partial and total cross sections on the scattering model and the accuracy of the target description is presented. The predicted angle-integrated elastic cross sections are in good agreement with experiment, whereas significant discrepancies are found in the angle-differential elastic cross sections near the forward direction. .The near-threshold results are found to strongly depend on the treatment of inner-core short-range correlation effects in the target description, as well as on a proper account of the target polarizability. A sharp increase in the elastic cross sections below 1 eV found in some earlier calculations is judged to be an artifact of an unbalanced description of correlation in the N-electron target structure and the (N+l)-electron-collision problems.
Total cross section of electron scattering by fluorocarbon molecules
NASA Astrophysics Data System (ADS)
Yamada, T.; Ushiroda, S.; Kondo, Y.
2008-12-01
A compact linear electron transmission apparatus was used for the measurement of the total electron scattering cross section at 4-500 eV. Total cross sections of chlorofluorocarbon (CCl2F2), hydrochlorofluorocarbon (CHClF2), perfluoropropane (C3F8), perfluoro-n-pentane (C5F12), perfluoro-n-hexane (C6F14) and perfluoro-n-octane (C8F18) were obtained experimentally and compared with the values obtained from a theoretical calculation and semi-empirical model calculation.
Townsend coefficients for electron scattering over dielectric surfaces
NASA Technical Reports Server (NTRS)
Peck, Timothy L.; Kushner, Mark J.
1988-01-01
A method for describing the probability of initiating flashover discharges across dielectric surfaces is presented in which a transport coefficient for electron multiplication similar to the Townsend coefficient used for gas discharges is defined. The coefficient is a function of the scaling parameter (charge released from the cathode)/(cathode-anode separation) and is also a measure of the growth of the sheath on the dielectric surface resulting from electron scattering. Results are discussed as to when the source of seed electrons does not necessarily depend upon field emission at the cathode-vacuum-dielectric triple point. For these conditions, there is a different functional dependence of flashover probability on voltage and geometry than when field emission provides the seed electrons. As a result, criteria previously used to predict flashover discharges may not apply.
Return Current Electron Beams and Their Generation of "Raman" Scattering
NASA Astrophysics Data System (ADS)
Simon, A.
1998-11-01
For some years, we(A. Simon and R. W. Short, Phys. Rev. Lett. 53), 1912 (1984). have proposed that the only reasonable explanation for many of the observations of "Raman" scattering is the presence of an electron beam in the plasma. (The beam creates a bump-on-tail instability.) Two major objections to this picture have been observation of Raman when no n_c/4 surface was present, with no likely source for the electron beam, and the necessity for the initially outward directed beam to bounce once to create the proper waves. Now new observations on LLE's OMEGA(R. Petrasso et al), this conference. and at LULI(C. Labaune et al)., Phys. Plasma 5, 234 (1998). have suggested a new origin for the electron beam. This new scenario answers the previous objections, maintains electron beams as the explanation of the older experiments, and may clear up puzzling observations that have remained unexplained. The new scenario is based on two assumptions: (1) High positive potentials develop in target plasmas during their creation. (2) A high-intensity laser beam initiates spark discharges from nearby surfaces to the target plasma. The resulting return current of electrons should be much more delta-like, is initially inwardly directed, and no longer requires the continued presence of a n_c/4 surface. Scattering of the interaction beam from the BOT waves yields the observed Raman signal. Experimental observations that support this picture will be cited. ``Pulsation'' of the scattering and broadband ``flashes'' are a natural part of this scenario. This work was supported by the U.S. Department of Energy Office of Inertial Confinement Fusion under Cooperative Agreement No. DE-FC03-92SF19460.
Optimization of Plasmon Decay Through Scattering and Hot Electron Transfer
NASA Astrophysics Data System (ADS)
DeJarnette, Drew
Light incident on metal nanoparticles induce localized surface oscillations of conductive electrons, called plasmons, which is a means to control and manipulate light. Excited plasmons decay as either thermal energy as absorbed phonons or electromagnetic energy as scattered photons. An additional decay pathway for plasmons can exist for gold nanoparticles situated on graphene. Excited plasmons can decay directly to the graphene as through hot electron transfer. This dissertation begins by computational analysis of plasmon resonance energy and bandwidth as a function of particle size, shape, and dielectric environment in addition to diffractive coupled in lattices creating a Fano resonance. With this knowledge, plasmon resonance was probed with incident electrons using electron energy loss spectroscopy in a transmission electron microscope. Nanoparticles were fabricated using electron beam lithography on 50 nanometer thick silicon nitride with some particles fabricated with a graphene layer between the silicon nitride and metal structure. Plasmon resonance was compared between ellipses on and off graphene to characterize hot electron transfer as a means of plasmon decay. It was observed that the presence of graphene caused plasmon energy to decrease by as much as 9.8% and bandwidth to increase by 25%. Assuming the increased bandwidth was solely from electron transfer as an additional plasmon decay route, a 20% efficiency of plasmon decay to graphene was calculated for the particular ellipses analyzed.
Elastic scattering of slow electrons by n-pentanol alcohol
NASA Astrophysics Data System (ADS)
de Oliveira, Eliane M.; Varella, Márcio T. do N.; Bettega, Márcio H. F.; Lima, Marco A. P.
2014-03-01
We report elastic integral (ICS), differential (DCS) and momentum transfer cross sections (MTCS) for low-energy electron scattering by n-pentanol alcohol in the gas phase. The Schwinger multichannel method implemented with pseudopotentials was employed in the calculations. The DCSs were computed for energies from 1 to 50 eV and the ICS and MTCS from 1 to 100 eV. Due to the significant value of the electric dipole moment, the DCSs are dominated by strong forward scattering. Despite this fact, the DCS around 10 eV displays a behavior related to a f-wave scattering pattern at intermediate angles which may be associated with shape resonances. This result is consistent with the ICS and the MTCS since they show a pronounced peak near this energy. For energies below 1 eV, the MTCS obtained in the static-exchange plus polarization approximation does not increase, as expected for polar molecules, suggesting that a Ramsauer-Townsend minimum could be present. This finding motivated us to revisit the previously studied methanol, ethanol, n-propanol and n-butanol molecules and to perform new calculations for impact energies below 1 eV (not addressed before). With the inclusion of polarization effects, the MTCS for the five alcohols suggest a Ramsauer-Townsend minimum coming from the negative to the positive scattering energies. To the best of our knowledge, there are neither experimental nor calculated cross sections for comparison with the present results.
Scattered data interpolation methods for electronic imaging systems: a survey
NASA Astrophysics Data System (ADS)
Amidror, Isaac
2002-04-01
Numerous problems in electronic imaging systems involve the need to interpolate from irregularly spaced data. One example is the calibration of color input/output devices with respect to a common intermediate objective color space, such as XYZ or L*a*b*. In the present report we survey some of the most important methods of scattered data interpolation in two-dimensional and in three-dimensional spaces. We review both single-valued cases, where the underlying function has the form f: R2 yields R or f: R3 yields R, and multivalued cases, where the underlying function is f: R2 yields R2 or f: R3 yields R3. The main methods we review include linear triangular (or tetrahedral) interpolation, cubic triangular (Clough--Tocher) interpolation, triangle based blending interpolation, inverse distance weighted methods, radial basis function methods, and natural neighbor interpolation methods. We also review one method of scattered data fitting, as an illustration to the basic differences between scattered data interpolation and scattered data fitting.
A Guide to Electronic Multipoles in Photon Scattering and Absorption
NASA Astrophysics Data System (ADS)
Lovesey, Stephen William; Balcar, Ewald
2013-02-01
The practice of replacing matrix elements in atomic calculations by those of convenient operators with strong physical appeal has a long history, and in condensed matter physics it is perhaps best known through use of operator equivalents in electron resonance by Elliott and Stevens. Likewise, electronic multipoles, created with irreducible spherical-tensors, to represent charge-like and magnetic-like quantities are widespread in modern physics. Examples in recent headlines include a magnetic charge (a monopole), an anapole (a dipole) and a triakontadipole (a magnetic-like atomic multipole of rank 5). In this communication, we aim to guide the reader through use of atomic, spherical multipoles in photon scattering, and resonant Bragg diffraction and dichroic signals in particular. Applications to copper oxide CuO and neptunium dioxide (NpO2) are described. In keeping with it being a simple guide, there is sparse use in the communication of algebra and expressions are gathered from the published literature and not derived, even when central to the exposition. An exception is a thorough grounding, contained in an Appendix, for an appropriate version of the photon scattering length based on quantum electrodynamics. A theme of the guide is application of symmetry in scattering, in particular constraints imposed on results by symmetry in crystals. To this end, a second Appendix catalogues constraints on multipoles imposed by symmetry in crystal point-groups.
Comparison between electron and neutron Compton scattering studies
NASA Astrophysics Data System (ADS)
Moreh, Raymond; Finkelstein, Yacov; Vos, Maarten
2015-05-01
We compare two techniques: Electron Compton Scattering (ECS) and neutron Compton scattering (NCS) and show that using certain incident energies, both can measure the atomic kinetic energy of atoms in molecules and solids. The information obtained is related to the Doppler broadening of nuclear levels and is very useful for deducing the widths of excited levels in many nuclei in self absorption measurements. A comparison between the atomic kinetic energies measured by the two methods on the same samples is made. Some results are also compared with calculated atomic kinetic energies obtained using the harmonic approximation where the vibrational frequencies were taken from IR/Raman optical measurements. The advantages of the ECS method are emphasized.
Elastic scattering of low-energy electrons from toluene
NASA Astrophysics Data System (ADS)
Sakaamini, Ahmad; Hargreaves, L. R.; Khakoo, M. A.; Pastega, D. F.; Bettega, M. H. F.
2016-04-01
Theoretical and normalized experimental differential, momentum transfer, and integral cross sections for vibrationally elastic scattering of low-energy electrons from toluene (C6H5C H3 ) are presented. The differential cross sections are measured at incident energies from 1 to 20 eV and scattering angles from 15° to 130°. The calculated cross sections are obtained using the Schwinger multichannel method with pseudopotentials in the static-exchange plus polarization approximation. Comparisons are made between the present theory and measurements with earlier available measurements. In general, the agreement between the theory and the experiment is very good. We also discuss the resonance spectra of toluene, where we find three π* shape resonances whose locations agree well with the experiment. In addition, we compare the cross sections of toluene and benzene, since the former can be considered as a benzene derivative by the substitution of a hydrogen in benzene by a C H3 group in toluene.
Electron scattering times in ZnO based polar heterostructures
Falson, J.; Kozuka, Y.; Smet, J. H.; Arima, T.; Tsukazaki, A.; Kawasaki, M.
2015-08-24
The remarkable historic advances experienced in condensed matter physics have been enabled through the continued exploration and proliferation of increasingly richer and cleaner material systems. In this work, we report on the scattering times of charge carriers confined in state-of-the-art MgZnO/ZnO heterostructures displaying electron mobilities in excess of 10{sup 6} cm{sup 2}/V s. Through an examination of low field quantum oscillations, we obtain the effective mass of charge carriers, along with the transport and quantum scattering times. These times compare favorably with high mobility AlGaAs/GaAs heterostructures, suggesting the quality of MgZnO/ZnO heterostructures now rivals that of traditional semiconductors.
NASA Astrophysics Data System (ADS)
Signorini, C.; Mazzocco, M.; Molini, P.; Pierroutsakou, D.; Boiano, C.; Manea, C.; Strano, E.; Torresi, D.; Di Meo, P.; Nicoletto, M.; Boiano, A.; Glodariu, T.; Grebosz, J.; Guglielmetti, A.; La Commara, M.; Parascandolo, C.; Parascandolo, L.; Sandoli, M.; Soramel, F.; Stroe, L.; Toniolo, N.; Veronese, F.
2013-03-01
The quasi elastic scattering of a 17O projectile from a 58Ni target has been studied at beam energies ranging from 42.5 to 55.0 MeV in 2.5 MeV steps. The total reaction cross sections were derived from the measured angular distributions by using an optical model fit within the coupled-channel code FRESCO. These cross sections are very similar to those measured for 17F (loosely bound by 0.6 MeV), mirror nucleus of 17O (tightly bound by 4.14 MeV). This outcome points out that, in this energy range, the small binding energy of the 17F valence proton has negligible influence onto the reactivity of such a loosely bound projectile, contrary to simple expectations, and to what observed for other loosely bound nuclei. The reaction dynamics seems to be influenced mainly by the Coulomb interaction which is similar for both mirror projectiles.
Practical correction procedures for elastic electron scattering effects in ARXPS
NASA Astrophysics Data System (ADS)
Lassen, T. S.; Tougaard, S.; Jablonski, A.
2001-06-01
Angle-resolved XPS and AES (ARXPS and ARAES) are widely used for determination of the in-depth distribution of elements in the surface region of solids. It is well known that elastic electron scattering has a significant effect on the intensity as a function of emission angle and that this has a great influence on the determined overlayer thicknesses by this method. However the applied procedures for ARXPS and ARAES generally neglect this because no simple and practical procedure for correction has been available. However recently, new algorithms have been suggested. In this paper, we have studied the efficiency of these algorithms to correct for elastic scattering effects in the interpretation of ARXPS and ARAES. This is done by first calculating electron distributions by Monte Carlo simulations for well-defined overlayer/substrate systems and then to apply the different algorithms. We have found that an analytical formula based on a solution of the Boltzmann transport equation provides a good account for elastic scattering effects. However this procedure is computationally very slow and the underlying algorithm is complicated. Another much simpler algorithm, proposed by Nefedov and coworkers, was also tested. Three different ways of handling the scattering parameters within this model were tested and it was found that this algorithm also gives a good description for elastic scattering effects provided that it is slightly modified so that it takes into account the differences in the transport properties of the substrate and the overlayer. This procedure is fairly simple and is described in detail. The model gives a much more accurate description compared to the traditional straight-line approximation (SLA). However it is also found that when attenuation lengths instead of inelastic mean free paths are used in the simple SLA formalism, the effects of elastic scattering are also reasonably well accounted for. Specifically, from a systematic study of several
NASA Technical Reports Server (NTRS)
Kumar, Vijay; Subramanian, K. P.; Krishnakumar, E.
1987-01-01
Absolute electron-helium and electron-neon scattering cross sections have been measured at low electron energies using the powerful technique of photoelectron spectroscopy. The measurements have been carried out at 17 electron energies varying from 0.7 to 10 eV with an accuracy of + or - 2.7 percent. The results obtained in the present work have been compared with other recent measurement and calculations.
Electron Scattering at Surfaces and Interfaces of Transition Metals
NASA Astrophysics Data System (ADS)
Zheng, Pengyuan
The effect of surfaces on the electron transport at reduced scales is attracting continuous interest due to its broad impact on both the understanding of materials properties and their application for nanoelectronics. The size dependence of for conductor's electrical resistivity rho due to electron surface scattering is most commonly described within the framework of Fuchs and Sondheimer (FS) and their various extensions, which uses a phenomenological scattering parameter p to define the probability of electrons being elastically (i.e. specularly) scattered by the surface without causing an increase of rho at reduced size. However, a basic understanding of what surface chemistry and structure parameters determine the specularity p is still lacking. In addition, the assumption of a spherical Fermi surface in the FS model is too simple for transition metals to give accurate account of the actual surface scattering effect. The goal of this study is to develop an understanding of the physics governing electron surface/interface scattering in transition metals and to study the significance of their Fermi surface shape on surface scattering. The advancement of the scientific knowledge in electron surface and interface scattering of transition metals can provide insights into how to design high-conductivity nanowires that will facilitate the viable development of advanced integrated circuits, thermoelectric power generation and spintronics. Sequential in situ and ex situ transport measurements as a function of surface chemistry demonstrate that electron surface/interface scattering can be engineered by surface doping, causing a decrease in the rho. For instance, the rho of 9.3-nm-thick epitaxial and polycrystalline Cu is reduced by 11--13% when coated with 0.75 nm Ni. This is due to electron surface scattering which exhibits a specularity p = 0.7 for the Cu-vacuum interface that transitions to completely diffuse (p = 0) when exposed to air. In contrast, Ni-coated surfaces
Quasi-Elastic Barrier Distribution for the {sup 7}Li+{sup 144}Sm Weakly Bound System
Otomar, D. R.; Gomes, P. R. S.; Lubian, J.; Monteiro, D. S.
2009-06-03
We have measured the excitation function of quasielastic and elastic scattering, at backward angles, for a range of energies from below to above the Coulomb barrier, for the {sup 7}Li+{sup 144}Sm system. Barrier distributions were exctracted from these excitation functions by a numerical method. From the theoretical analysis one concluded that the quadrupole and octupole excitations of {sup 144}Sm and the one-neutron transfer (stripping) channel are important reaction processes. Nevertheless, the agreement with the experimental results is poor. The discrepancy is attributed to the {sup 7}Li break-up channel that was not taken into account in the coupling scheme.
Scattering of positrons and electrons by alkali atoms
NASA Technical Reports Server (NTRS)
Stein, T. S.; Kauppila, W. E.; Kwan, C. K.; Lukaszew, R. A.; Parikh, S. P.; Wan, Y. J.; Zhou, S.; Dababneh, M. S.
1990-01-01
Absolute total scattering cross sections (Q sub T's) were measured for positrons and electrons colliding with sodium, potassium, and rubidium in the 1 to 102 eV range, using the same apparatus and experimental approach (a beam transmission technique) for both projectiles. The present results for positron-sodium and -rubidium collisions represent the first Q sub T measurements reported for these collision systems. Features which distinguish the present comparisons between positron- and electron-alkali atom Q sub T's from those for other atoms and molecules (room-temperature gases) which have been used as targets for positrons and electrons are the proximity of the corresponding positron- and electron-alkali atom Q sub T's over the entire energy range of overlap, with an indication of a merging or near-merging of the corresponding positron and electron Q sub T's near (and above) the relatively low energy of about 40 eV, and a general tendency for the positron-alkali atom Q sub T's to be higher than the corresponding electron values as the projectile energy is decreased below about 40 eV.
Measurement of parity violation in electron-quark scattering
NASA Astrophysics Data System (ADS)
The Jefferson Lab Pvdis Collaboration; Wang, D.; Pan, K.; Subedi, R.; Deng, X.; Ahmed, Z.; Allada, K.; Aniol, K. A.; Armstrong, D. S.; Arrington, J.; Bellini, V.; Beminiwattha, R.; Benesch, J.; Benmokhtar, F.; Bertozzi, W.; Camsonne, A.; Canan, M.; Cates, G. D.; Chen, J.-P.; Chudakov, E.; Cisbani, E.; Dalton, M. M.; de Jager, C. W.; de Leo, R.; Deconinck, W.; Deur, A.; Dutta, C.; El Fassi, L.; Erler, J.; Flay, D.; Franklin, G. B.; Friend, M.; Frullani, S.; Garibaldi, F.; Gilad, S.; Giusa, A.; Glamazdin, A.; Golge, S.; Grimm, K.; Hafidi, K.; Hansen, J.-O.; Higinbotham, D. W.; Holmes, R.; Holmstrom, T.; Holt, R. J.; Huang, J.; Hyde, C. E.; Jen, C. M.; Jones, D.; Kang, Hoyoung; King, P. M.; Kowalski, S.; Kumar, K. S.; Lee, J. H.; Lerose, J. J.; Liyanage, N.; Long, E.; McNulty, D.; Margaziotis, D. J.; Meddi, F.; Meekins, D. G.; Mercado, L.; Meziani, Z.-E.; Michaels, R.; Mihovilovic, M.; Muangma, N.; Myers, K. E.; Nanda, S.; Narayan, A.; Nelyubin, V.; Nuruzzaman; Oh, Y.; Parno, D.; Paschke, K. D.; Phillips, S. K.; Qian, X.; Qiang, Y.; Quinn, B.; Rakhman, A.; Reimer, P. E.; Rider, K.; Riordan, S.; Roche, J.; Rubin, J.; Russo, G.; Saenboonruang, K.; Saha, A.; Sawatzky, B.; Shahinyan, A.; Silwal, R.; Sirca, S.; Souder, P. A.; Suleiman, R.; Sulkosky, V.; Sutera, C. M.; Tobias, W. A.; Urciuoli, G. M.; Waidyawansa, B.; Wojtsekhowski, B.; Ye, L.; Zhao, B.; Zheng, X.
2014-02-01
Symmetry permeates nature and is fundamental to all laws of physics. One example is parity (mirror) symmetry, which implies that flipping left and right does not change the laws of physics. Laws for electromagnetism, gravity and the subatomic strong force respect parity symmetry, but the subatomic weak force does not. Historically, parity violation in electron scattering has been important in establishing (and now testing) the standard model of particle physics. One particular set of quantities accessible through measurements of parity-violating electron scattering are the effective weak couplings C2q, sensitive to the quarks' chirality preference when participating in the weak force, which have been measured directly only once in the past 40years. Here we report a measurement of the parity-violating asymmetry in electron-quark scattering, which yields a determination of 2C2u-C2d (where u and d denote up and down quarks, respectively) with a precision increased by a factor of five relative to the earlier result. These results provide evidence with greater than 95 per cent confidence that the C2q couplings are non-zero, as predicted by the electroweak theory. They lead to constraints on new parity-violating interactions beyond the standard model, particularly those due to quark chirality. Whereas contemporary particle physics research is focused on high-energy colliders such as the Large Hadron Collider, our results provide specific chirality information on electroweak theory that is difficult to obtain at high energies. Our measurement is relatively free of ambiguity in its interpretation, and opens the door to even more precise measurements in the future.
Measurement of parity violation in electron-quark scattering.
2014-02-01
Symmetry permeates nature and is fundamental to all laws of physics. One example is parity (mirror) symmetry, which implies that flipping left and right does not change the laws of physics. Laws for electromagnetism, gravity and the subatomic strong force respect parity symmetry, but the subatomic weak force does not. Historically, parity violation in electron scattering has been important in establishing (and now testing) the standard model of particle physics. One particular set of quantities accessible through measurements of parity-violating electron scattering are the effective weak couplings C2q, sensitive to the quarks' chirality preference when participating in the weak force, which have been measured directly only once in the past 40 years. Here we report a measurement of the parity-violating asymmetry in electron-quark scattering, which yields a determination of 2C2u - C2d (where u and d denote up and down quarks, respectively) with a precision increased by a factor of five relative to the earlier result. These results provide evidence with greater than 95 per cent confidence that the C2q couplings are non-zero, as predicted by the electroweak theory. They lead to constraints on new parity-violating interactions beyond the standard model, particularly those due to quark chirality. Whereas contemporary particle physics research is focused on high-energy colliders such as the Large Hadron Collider, our results provide specific chirality information on electroweak theory that is difficult to obtain at high energies. Our measurement is relatively free of ambiguity in its interpretation, and opens the door to even more precise measurements in the future. PMID:24499917
Elastic Scattering of Low-Energy Electrons byTetrahydrofuran
Trevisan, Cynthia S.; Orel, Ann E.; Rescigno, Thomas N.
2006-05-09
We present the results of ab initio calculations for elasticelectron scattering by tetrahydrofuran (THF) using the complex Kohnvariational method. We carried out fixed-nuclei calculations at theequilibrium geometry of the target molecule for incident electronenergies up to 20 eV. The calculated momentum transfer cross sectionsclearly reveal the presence of broad shape resonance behavior in the 8-10eV energy range, in agreement with recent experiments. The calculateddifferential cross sections at 20 eV, which include the effects of thelong-range electron-dipole interaction, are alsofound to be in agreementwith the most recent experimental findings.
Consistency of electron scattering data with a small proton radius
NASA Astrophysics Data System (ADS)
Griffioen, Keith; Carlson, Carl; Maddox, Sarah
2016-06-01
We determine the charge radius of the proton by analyzing the published low momentum transfer electron-proton scattering data from Mainz. We note that polynomial expansions of the form factor converge for momentum transfers squared below 4 mπ2 , where mπ is the pion mass. Expansions with enough terms to fit the data, but few enough not to overfit, yield proton radii smaller than the CODATA or Mainz values and in accord with the muonic atom results. We also comment on analyses using a wider range of data, and overall obtain a proton radius RE=0.840 (16 ) fm.
Transition probability functions for applications of inelastic electron scattering.
Löffler, Stefan; Schattschneider, Peter
2012-09-01
In this work, the transition matrix elements for inelastic electron scattering are investigated which are the central quantity for interpreting experiments. The angular part is given by spherical harmonics. For the weighted radial wave function overlap, analytic expressions are derived in the Slater-type and the hydrogen-like orbital models. These expressions are shown to be composed of a finite sum of polynomials and elementary trigonometric functions. Hence, they are easy to use, require little computation time, and are significantly more accurate than commonly used approximations. PMID:22560709
Results on neutrino-electron elastic scattering at AGS energies
Lanou, R.E.
1984-02-26
In an experiment designed to study elastic scattering of nu/sub ..mu../ (and anti nu/sub ..mu../) from electrons and protons via the weak neutral current, we have recently completed several extensive data taking runs. Results for the cross section of nu/sub ..mu../ + e/sup -/ ..-->.. nu/sub ..mu../ + e/sup -/ are presented based upon the first third of the available sample. Preliminary analysis of anti nu/sub ..mu../ + e/sup -/ ..-->.. anti nu/sub ..mu../ + e/sup -/ is in progress and evidence for the signal is presented.
Scattered electron beams shaped by a multileaf collimator
NASA Astrophysics Data System (ADS)
Moran, Jean Marie
Recent developments in conformal radiation therapy have focused primarily on applying computer-controlled equipment and techniques to photon beams. Despite favorable characteristics of the dose fall-off with depth for electron beams, their application to conformal therapy has been limited. Factors such as geometrically limiting applicator systems, lack of automatic field shaping, and dose calculation model limitations must be addressed before routine clinical use of electron beams for conformal radiotherapy becomes common. This work evaluates dose characteristics and modeling of dose distributions and output factors for a system specifically designed for computer-controlled collimation of dual-foil scattered and scanned electron beams. Dose characteristics determined from measured depth dose curves and profiles were evaluated for multileaf- collimated and applicator-collimated beams produced by the dual-foil scattered gantry of a two-gantry racetrack microtron system. The resulting dose distributions and characteristics were used to evaluate and modify the existing 3-D electron pencil beam algorithm in UMPlan, the University of Michigan treatment planning system, to predict relative dose distributions for MLC-shaped fields. Output factors (dose of a field relative to that of a reference field) were measured, analyzed, and modeled for MLC-collimated rectangular and shaped fields. For output factor calculations, two models were evaluated: a pencil beam-derived model and an empirical edge model originally developed for photon dose calculations. The current work shows that the dosimetric characteristics of MLC and applicator-collimated beams of the racetrack microtron are similar once the collimation geometry is accounted for. The dosimetric characteristics are also consistent with those for other dual-foil scattered machines with applicator systems and earlier generation scanned beams collimated with trimmer bars. By accounting for collimation geometry, electron
Electronic scattering effects in europium-based iron pnictides
NASA Astrophysics Data System (ADS)
Zapf, Sina; Neubauer, David; Post, Kirk W.; Kadau, Alina; Merz, Johannes; Clauss, Conrad; Löhle, Anja; Jeevan, Hirale S.; Gegenwart, Philipp; Basov, Dimitri N.; Dressel, Martin
2016-01-01
In a comprehensive study, we investigate the electronic scattering effects in EuFe2(As1-xPx) 2 by using Fourier-transform infrared spectroscopy. In spite of the fact that Eu2+ local moments order at around TEu ∼ 20 K, the overall optical response is strikingly similar to the one of the well-known Ba-122 pnictides. The main difference lies within the suppression of the lower spin-density-wave gap feature. By analyzing our spectra with a multi-component model, we find that the high-energy feature around 0.7 eV - often associated with Hund's rule coupling - is highly sensitive to the spin-density-wave ordering; this further confirms its direct relationship to the dynamics of itinerant carriers. The same model is also used to investigate the in-plane anisotropy of magnetically detwinned EuFe2As2 in the antiferromagnetically ordered state, yielding a higher Drude weight and lower scattering rate along the crystallographic a-axis. Finally, we analyze the development of the room-temperature spectra with isovalent phosphor substitution and highlight changes in the scattering rate of hole-like carriers induced by a Lifshitz transition.
NASA Astrophysics Data System (ADS)
Tretiak, Sergei
2014-03-01
The exciton scattering (ES) technique is a multiscale approach developed for efficient calculations of excited-state electronic structure and optical spectra in low-dimensional conjugated macromolecules. Within the ES method, the electronic excitations in the molecular structure are attributed to standing waves representing quantum quasi-particles (excitons), which reside on the graph. The exciton propagation on the linear segments is characterized by the exciton dispersion, whereas the exciton scattering on the branching centers is determined by the energy-dependent scattering matrices. Using these ES energetic parameters, the excitation energies are then found by solving a set of generalized ``particle in a box'' problems on the graph that represents the molecule. All parameters can be extracted from quantum-chemical computations of small molecular fragments and tabulated in the ES library for further applications. Subsequently, spectroscopic modeling for any macrostructure within considered molecular family could be performed with negligible numerical effort. The exciton scattering properties of molecular vertices can be further described by tight-binding or equivalently lattice models. The on-site energies and hopping constants are obtained from the exciton dispersion and scattering matrices. Such tight-binding model approach is particularly useful to describe the exciton-phonon coupling, energetic disorder and incoherent energy transfer in large branched conjugated molecules. Overall the ES applications accurately reproduce the optical spectra compared to the reference quantum chemistry results, and make possible to predict spectra of complex macromolecules, where conventional electronic structure calculations are unfeasible.