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Sample records for resonant optical phonon

  1. Confined optical-phonon-assisted cyclotron resonance in quantum wells via two-photon absorption process

    NASA Astrophysics Data System (ADS)

    Phuc, Huynh Vinh; Hien, Nguyen Dinh; Dinh, Le; Phong, Tran Cong

    2016-06-01

    The effect of confined phonons on the phonon-assisted cyclotron resonance (PACR) via both one and two photon absorption processes in a quantum well is theoretically studied. We consider cases when electrons are scattered by confined optical phonons described by the Fuchs-Kliewer slab, Ridley's guided, and Huang-Zhu models. The analytical expression of the magneto-optical absorption coefficient (MOAC) is obtained by relating it to the transition probability for the absorption of photons. It predicts resonant peaks caused by transitions between Landau levels and electric subband accompanied by confined phonons emission in the absorption spectrum. The MOAC and the full-width at half-maximum (FWHM) for the intra- and inter-subband transitions are given as functions of the magnetic field, temperature, and quantum well width. In narrow quantum wells, the phonon confinement becomes more important and should be taken into account in studying FWHM.

  2. Evidence of longitudinal resonance and optical subsurface phonons in Al(001)

    NASA Astrophysics Data System (ADS)

    Chis, Vasile; Hellsing, Bo; Benedek, Giorgio; Bernasconi, Marco; Toennies, J. P.

    2007-08-01

    A calculation of the surface phonon dispersion curves of Al(001) based on density functional perturbation theory confirms the intrinsic nature of the controversial longitudinal surface phonon resonance, which has been reported to occur in most metal surfaces. The results support previous density-response pseudopotential and semi-empirical Born-von-Kàrmàn calculations by Franchini, Bortolani, et al, proving the extended nature of the surface perturbation. The latter implies the existence of a Lucas pair of optical surface modes localized in the second layer.

  3. Optical and acoustic sensing using Fano-like resonances in dual phononic and photonic crystal plate

    NASA Astrophysics Data System (ADS)

    Amoudache, Samira; Moiseyenko, Rayisa; Pennec, Yan; Rouhani, Bahram Djafari; Khater, Antoine; Lucklum, Ralf; Tigrine, Rachid

    2016-03-01

    We perform a theoretical study based on the transmissions of optical and acoustic waves normally impinging to a periodic perforated silicon plate when the embedded medium is a liquid and show the existence of Fano-like resonances in both cases. The signature of the resonances appears as well-defined asymmetric peaks in the phononic and photonic transmission spectra. We show that the origin of the Fano-like resonances is different with respect to the nature of the wave. In photonic, the origin comes from guided modes in the photonic plate while in phononic we show that it comes from the excitation of standing waves confined inside the cavity coming from the deformation of the water/silicon edges of the cylindrical inclusion. We finally use these features for sensing and show ultra-sensitivity to the light and sound velocities for different concentrations of analytes.

  4. Resonant raman scattering and dispersion of polar optical and acoustic phonons in hexagonal inn

    SciTech Connect

    Davydov, V. Yu. Klochikhin, A. A.; Smirnov, A. N.; Strashkova, I. Yu.; Krylov, A. S.; Lu Hai; Schaff, William J.; Lee, H.-M.; Hong, Y.-L.; Gwo, S.

    2010-02-15

    It is shown that a study of the dependence of impurity-related resonant first-order Raman scattering on the frequency of excitation light makes it possible to observe the dispersion of polar optical and acoustic branches of vibrational spectrum in hexagonal InN within a wide range of wave vectors. It is established that the wave vectors of excited phonons are uniquely related to the energy of excitation photon. Frequencies of longitudinal optical phonons E{sub 1}(LO) and A{sub 1}(LO) in hexagonal InN were measured in the range of excitation-photon energies from 2.81 to 1.17 eV and the frequencies of longitudinal acoustic phonons were measured in the range 2.81-1.83 eV of excitation-photon energies. The obtained dependences made it possible to extrapolate the dispersion of phonons A{sub 1}(LO) and E{sub 1}(LO) to as far as the point {Gamma} in the Brillouin zone and estimate the center-band energies of these phonons (these energies have not been uniquely determined so far).

  5. Optical properties of single infrared resonant circular microcavities for surface phonon polaritons.

    PubMed

    Wang, Tao; Li, Peining; Hauer, Benedikt; Chigrin, Dmitry N; Taubner, Thomas

    2013-11-13

    Plasmonic antennas are crucial components for nano-optics and have been extensively used to enhance sensing, spectroscopy, light emission, photodetection, and others. Recently, there is a trend to search for new plasmonic materials with low intrinsic loss at new plasmon frequencies. As an alternative to metals, polar crystals have a negative real part of permittivity in the Reststrahlen band and support surface phonon polaritons (SPhPs) with weak damping. Here, we experimentally demonstrate the resonance of single circular microcavities in a thin gold film deposited on a silicon carbide (SiC) substrate in the mid-infrared range. Specifically, the negative permittivity of SiC leads to a well-defined, size-tunable SPhP resonance with a Q factor of around 60 which is much higher than those in surface plasmon polariton (SPP) resonators with similar structures. These infrared resonant microcavities provide new possibilities for widespread applications such as enhanced spectroscopy, sensing, coherent thermal emission, and infrared photodetectors among others throughout the infrared frequency range. PMID:24117024

  6. Terahertz lasers and amplifiers based on resonant optical phonon scattering to achieve population inversion

    NASA Technical Reports Server (NTRS)

    Hu, Qing (Inventor); Williams, Benjamin S. (Inventor)

    2007-01-01

    The present invention provides quantum cascade lasers and amplifier that operate in a frequency range of about 1 Terahertz to about 10 Terahertz. In one aspect, a quantum cascade laser of the invention includes a semiconductor heterostructure that provides a plurality of lasing modules connected in series. Each lasing module includes a plurality of quantum well structure that collectively generate at least an upper lasing state, a lower lasing state, and a relaxation state such that the upper and the lower lasing states are separated by an energy corresponding to an optical frequency in a range of about 1 to about 10 Terahertz. The lower lasing state is selectively depopulated via resonant LO-phonon scattering of electrons into the relaxation state.

  7. Terahertz lasers and amplifiers based on resonant optical phonon scattering to achieve population inversion

    NASA Technical Reports Server (NTRS)

    Hu, Qing (Inventor); Williams, Benjamin S. (Inventor)

    2009-01-01

    The present invention provides quantum cascade lasers and amplifier that operate in a frequency range of about 1 Terahertz to about 10 Terahertz. In one aspect, a quantum cascade laser of the invention includes a semiconductor heterostructure that provides a plurality of lasing modules connected in series. Each lasing module includes a plurality of quantum well structure that collectively generate at least an upper lasing state, a lower lasing state, and a relaxation state such that the upper and the lower lasing states are separated by an energy corresponding to an optical frequency in a range of about 1 to about 10 Terahertz. The lower lasing state is selectively depopulated via resonant LO-phonon scattering of electrons into the relaxation state.

  8. Phonon Josephson junction with nanomechanical resonators

    NASA Astrophysics Data System (ADS)

    Barzanjeh, Shabir; Vitali, David

    2016-03-01

    We study coherent phonon oscillations and tunneling between two coupled nonlinear nanomechanical resonators. We show that the coupling between two nanomechanical resonators creates an effective phonon Josephson junction, which exhibits two different dynamical behaviors: Josephson oscillation (phonon-Rabi oscillation) and macroscopic self-trapping (phonon blockade). Self-trapping originates from mechanical nonlinearities, meaning that when the nonlinearity exceeds its critical value, the energy exchange between the two resonators is suppressed, and phonon Josephson oscillations between them are completely blocked. An effective classical Hamiltonian for the phonon Josephson junction is derived and its mean-field dynamics is studied in phase space. Finally, we study the phonon-phonon coherence quantified by the mean fringe visibility, and show that the interaction between the two resonators may lead to the loss of coherence in the phononic junction.

  9. Resonant surface-enhanced Raman scattering by optical phonons in a monolayer of CdSe nanocrystals on Au nanocluster arrays

    NASA Astrophysics Data System (ADS)

    Milekhin, Alexander G.; Sveshnikova, Larisa L.; Duda, Tatyana A.; Rodyakina, Ekaterina E.; Dzhagan, Volodymyr M.; Sheremet, Evgeniya; Gordan, Ovidiu D.; Himcinschi, Cameliu; Latyshev, Alexander V.; Zahn, Dietrich R. T.

    2016-05-01

    Here we present the results on an investigation of resonant Stokes and anti- Stokes surface-enhanced Raman scattering (SERS) by optical phonons in colloidal CdSe nanocrystals (NCs) homogeneously deposited on arrays of Au nanoclusters using the Langmuir-Blodgett technology. The thickness of deposited NCs, determined by transmission and scanning electron microscopy, amounts to approximately 1 monolayer. Special attention is paid to the determination of the localized surface plasmon resonance (LSPR) energy in the arrays of Au nanoclusters as a function of the nanocluster size by means of micro-ellipsometry. SERS by optical phonons in CdSe NCs shows a significant enhancement factor with a maximal value of 2 × 103 which depends resonantly on the Au nanocluster size and thus on the LSPR energy. The deposition of CdSe NCs on the arrays of Au nanocluster dimers enabled us to study the polarization dependence of SERS. It was found that a maximal SERS signal is observed for the light polarization along the dimer axis. Finally, SERS by optical phonons was observed for CdSe NCs deposited on the structures with a single Au dimer. A difference of the LO phonon energy is observed for CdSe NCs on different single dimers. This effect is explained as the confinement-induced shift which depends on the CdSe nanocrystal size and indicates quasi-single NC Raman spectra being obtained.

  10. Temperature-dependent exciton resonance energies and their correlation with IR-active optical phonon modes in β-Ga2O3 single crystals

    NASA Astrophysics Data System (ADS)

    Onuma, T.; Saito, S.; Sasaki, K.; Goto, K.; Masui, T.; Yamaguchi, T.; Honda, T.; Kuramata, A.; Higashiwaki, M.

    2016-03-01

    Temperature-dependent exciton resonance energies Eexciton in β-Ga2O3 single crystals are studied by using polarized reflectance measurement. The Eexciton values exhibit large energy changes in the range of 179-268 meV from 5 to 300 K. The IR-active Au and Bu optical phonon modes are selectively observed in the IR spectroscopic ellipsometry spectra by reflecting the polarization selection rules. The longitudinal optical (LO) phonon energies can be divided into three ranges: ℏωLO = 35-48, 70-73, and 88-99 meV. The broadening parameters, which are obtained from the reflectance measurements, correspond to the lower two ranges of ℏωLO at low temperature and 75 meV above 150 K. The large Eexciton changes with temperature in β-Ga2O3 are found to be originated from the exciton-LO-phonon interaction.

  11. Optically driven quantum dots as source of coherent cavity phonons: a proposal for a phonon laser scheme.

    PubMed

    Kabuss, Julia; Carmele, Alexander; Brandes, Tobias; Knorr, Andreas

    2012-08-01

    We present a microscopically based scheme for the generation of coherent cavity phonons (phonon laser) by an optically driven semiconductor quantum dot coupled to a THz acoustic nanocavity. External laser pump light on an anti-Stokes resonance creates an effective Lambda system within a two-level dot that leads to coherent phonon statistics. We use an inductive equation of motion method to estimate a realistic parameter range for an experimental realization of such phonon lasers. This scheme for the creation of nonequilibrium phonons is robust with respect to radiative and phononic damping and only requires optical Rabi frequencies of the order of the electron-phonon coupling strength. PMID:23006175

  12. Resonant squeezing and the anharmonic decay of coherent phonons

    NASA Astrophysics Data System (ADS)

    Fahy, Stephen; Murray, Éamonn D.; Reis, David A.

    2016-04-01

    We show that the anharmonic decay of large-amplitude coherent phonons in a solid generates strongly enhanced squeezing of the phonon modes near points of the Brillouin zone where energy conservation in the three-phonon decay process is satisfied. The squeezing process leads to temporal oscillations of the mean-square displacement of target modes in resonance with the coherent phonon, which are characteristic of coherent phonon decay and do not occur in the decay of a phonon in a well-defined number state. For realistic material parameters of optically excited group-V semimetals, we predict that this squeezing results in strongly enhanced oscillations of the x-ray diffuse scattering intensity at sharply defined values of the x-ray momentum transfer. Numerical simulations of the phonon dynamics and the x-ray diffuse scattering in optically excited bismuth, using harmonic and anharmonic force parameters calculated with constrained density functional theory, demonstrate oscillations of the diffuse scattering intensity of magnitude 10%-20% of the thermal background at points of the Brillouin zone, where resonance occurs. Such oscillations should be observable using time-resolved optical-pump and x-ray-probe facilities available at current x-ray free-electron laser sources.

  13. Optical resonator

    NASA Technical Reports Server (NTRS)

    Taghavi-Larigani, Shervin (Inventor); Vanzyl, Jakob J. (Inventor); Yariv, Amnon (Inventor)

    2006-01-01

    The invention discloses a semi-ring Fabry-Perot (SRFP) optical resonator structure comprising a medium including an edge forming a reflective facet and a waveguide within the medium, the waveguide having opposing ends formed by the reflective facet. The performance of the SRFP resonator can be further enhanced by including a Mach-Zehnder interferometer in the waveguide on one side of the gain medium. The optical resonator can be employed in a variety of optical devices. Laser structures using at least one SRFP resonator are disclosed where the resonators are disposed on opposite sides of a gain medium. Other laser structures employing one or more resonators on one side of a gain region are also disclosed.

  14. Resonant and nonlocal properties of phononic metasolids

    NASA Astrophysics Data System (ADS)

    Torrent, Daniel; Pennec, Yan; Djafari-Rouhani, Bahram

    2015-11-01

    We derive a general theory of effective properties in metasolids based on phononic crystals with low frequency resonances. We demonstrate that in general these structures need to be described by means of a frequency-dependent and nonlocal anisotropic mass density, stiffness tensor and a third-rank coupling tensor, which shows that they behave like a nonlocal Willis medium. The effect of nonlocality and coupling tensor manifest themselves for some particular resonances, whereas they become negligible for other resonances. Considering the example of a two-dimensional phononic crystal, consisting of triangular arrangements of cylindrical shells in an elastic matrix, we show that its mass density tensor is strongly resonant and anisotropic presenting both positive and negative divergent values, while becoming scalar in the quasistatic limit. Moreover, it is found that the negative value of transverse component of the mass density is induced by a dipolar resonance, while that of the vertical component is induced by a monopolar one. Finally, the dispersion relation obtained by the effective parameters of the crystal is compared with the band structure, showing good agreement for the low-wave-number region, although the nonlocal effects are important given the existence of some resonant values of the wave number.

  15. Phonon-Assisted Resonant Tunnelling through a Triple-Quantum-Dot: a Phonon-Signal Detector

    NASA Astrophysics Data System (ADS)

    Shen, Xiao-Yun; Dong, Bing; Lei, Xiao-lin

    2008-02-01

    We study the effect of electron-phonon interaction on current and zero-frequency shot noise in resonant tunnelling through a series triple-quantum-dot coupling to a local phonon mode by means of a nonperturbative mapping technique along with the Green function formulation. By fixing the energy difference between the first two quantum dots to be equal to phonon frequency and sweeping the level of the third quantum dot, we find a largely enhanced current spectrum due to phonon effect, and in particular we predict current peaks corresponding to phonon-absorption and phonon-emission assisted resonant tunnelling processes, which show that this system can be acted as a sensitive phonon-signal detector or as a cascade phonon generator.

  16. Phonon-tunnelling dissipation in mechanical resonators

    PubMed Central

    Cole, Garrett D.; Wilson-Rae, Ignacio; Werbach, Katharina; Vanner, Michael R.; Aspelmeyer, Markus

    2011-01-01

    Microscale and nanoscale mechanical resonators have recently emerged as ubiquitous devices for use in advanced technological applications, for example, in mobile communications and inertial sensors, and as novel tools for fundamental scientific endeavours. Their performance is in many cases limited by the deleterious effects of mechanical damping. In this study, we report a significant advancement towards understanding and controlling support-induced losses in generic mechanical resonators. We begin by introducing an efficient numerical solver, based on the 'phonon-tunnelling' approach, capable of predicting the design-limited damping of high-quality mechanical resonators. Further, through careful device engineering, we isolate support-induced losses and perform a rigorous experimental test of the strong geometric dependence of this loss mechanism. Our results are in excellent agreement with the theory, demonstrating the predictive power of our approach. In combination with recent progress on complementary dissipation mechanisms, our phonon-tunnelling solver represents a major step towards accurate prediction of the mechanical quality factor. PMID:21407197

  17. Phonon counting and intensity interferometry of a nanomechanical resonator

    NASA Astrophysics Data System (ADS)

    Cohen, Justin D.; Meenehan, Seán M.; Maccabe, Gregory S.; Gröblacher, Simon; Safavi-Naeini, Amir H.; Marsili, Francesco; Shaw, Matthew D.; Painter, Oskar

    2015-04-01

    In optics, the ability to measure individual quanta of light (photons) enables a great many applications, ranging from dynamic imaging within living organisms to secure quantum communication. Pioneering photon counting experiments, such as the intensity interferometry performed by Hanbury Brown and Twiss to measure the angular width of visible stars, have played a critical role in our understanding of the full quantum nature of light. As with matter at the atomic scale, the laws of quantum mechanics also govern the properties of macroscopic mechanical objects, providing fundamental quantum limits to the sensitivity of mechanical sensors and transducers. Current research in cavity optomechanics seeks to use light to explore the quantum properties of mechanical systems ranging in size from kilogram-mass mirrors to nanoscale membranes, as well as to develop technologies for precision sensing and quantum information processing. Here we use an optical probe and single-photon detection to study the acoustic emission and absorption processes in a silicon nanomechanical resonator, and perform a measurement similar to that used by Hanbury Brown and Twiss to measure correlations in the emitted phonons as the resonator undergoes a parametric instability formally equivalent to that of a laser. Owing to the cavity-enhanced coupling of light with mechanical motion, this effective phonon counting technique has a noise equivalent phonon sensitivity of 0.89 +/- 0.05. With straightforward improvements to this method, a variety of quantum state engineering tasks using mesoscopic mechanical resonators would be enabled, including the generation and heralding of single-phonon Fock states and the quantum entanglement of remote mechanical elements.

  18. Phonon counting and intensity interferometry of a nanomechanical resonator.

    PubMed

    Cohen, Justin D; Meenehan, Seán M; MacCabe, Gregory S; Gröblacher, Simon; Safavi-Naeini, Amir H; Marsili, Francesco; Shaw, Matthew D; Painter, Oskar

    2015-04-23

    In optics, the ability to measure individual quanta of light (photons) enables a great many applications, ranging from dynamic imaging within living organisms to secure quantum communication. Pioneering photon counting experiments, such as the intensity interferometry performed by Hanbury Brown and Twiss to measure the angular width of visible stars, have played a critical role in our understanding of the full quantum nature of light. As with matter at the atomic scale, the laws of quantum mechanics also govern the properties of macroscopic mechanical objects, providing fundamental quantum limits to the sensitivity of mechanical sensors and transducers. Current research in cavity optomechanics seeks to use light to explore the quantum properties of mechanical systems ranging in size from kilogram-mass mirrors to nanoscale membranes, as well as to develop technologies for precision sensing and quantum information processing. Here we use an optical probe and single-photon detection to study the acoustic emission and absorption processes in a silicon nanomechanical resonator, and perform a measurement similar to that used by Hanbury Brown and Twiss to measure correlations in the emitted phonons as the resonator undergoes a parametric instability formally equivalent to that of a laser. Owing to the cavity-enhanced coupling of light with mechanical motion, this effective phonon counting technique has a noise equivalent phonon sensitivity of 0.89 ± 0.05. With straightforward improvements to this method, a variety of quantum state engineering tasks using mesoscopic mechanical resonators would be enabled, including the generation and heralding of single-phonon Fock states and the quantum entanglement of remote mechanical elements. PMID:25903632

  19. Evolution of molecular crystal optical phonons near structural phase transitions

    NASA Astrophysics Data System (ADS)

    Michki, Nigel; Niessen, Katherine; Xu, Mengyang; Markelz, Andrea

    Molecular crystals are increasingly important photonic and electronic materials. For example organic semiconductors are lightweight compared to inorganic semiconductors and have inexpensive scale up processing with roll to roll printing. However their implementation is limited by their environmental sensitivity, in part arising from the weak intermolecular interactions of the crystal. These weak interactions result in optical phonons in the terahertz frequency range. We examine the evolution of intermolecular interactions near structural phase transitions by measuring the optical phonons as a function of temperature and crystal orientation using terahertz time-domain spectroscopy. The measured orientation dependence of the resonances provides an additional constraint for comparison of the observed spectra with the density functional calculations, enabling us to follow specific phonon modes. We observe crystal reorganization near 350 K for oxalic acid as it transforms from dihydrate to anhydrous form. We also report the first THz spectra for the molecular crystal fructose through its melting point.

  20. Structure-Dependent Fano Resonances in the Infrared Spectra of Phonons in Few-Layer Graphene

    SciTech Connect

    Li Z.; Carr G.; Chun Hung,L.; Cappelluti, E.; Benfatto, L.; Mak, K.F.; Jie, S.; Heinz, T.F.

    2012-04-10

    The in-plane optical phonons around 200 meV in few-layer graphene are investigated utilizing infrared absorption spectroscopy. The phonon spectra exhibit unusual asymmetric features characteristic of Fano resonances, which depend critically on the layer thickness and stacking order of the sample. The phonon intensities in samples with rhombohedral (ABC) stacking are significantly higher than those with Bernal (AB) stacking. These observations reflect the strong coupling between phonons and interband electronic transitions in these systems and the distinctive variation in the joint density of electronic states in samples of differing thickness and stacking order.

  1. Optical phonon modes in ordered core-shell CdSe/CdS nanorod arrays

    NASA Astrophysics Data System (ADS)

    Giugni, Andrea; Das, Gobind; Alabastri, Alessandro; Zaccaria, Remo Proietti; Zanella, Marco; Franchini, Isabella; di Fabrizio, Enzo; Krahne, Roman

    2012-03-01

    We investigate the optical phonons in “dot-in-a-rod” core-shell CdSe/CdS nanorods at wavelengths resonant with the optical transitions either in the core or in the shell. At a wavelength above the CdS band gap, only CdS phonon modes were detected. In contrast, at excitation in resonance with the core transitions, we observed phonon modes of both the CdSe core and the CdS shell. In laterally ordered nanorod assemblies, the CdS longitudinal-optical phonon mode manifested a low-energy shoulder that could be related to higher-order longitudinal-optical phonon modes. Furthermore, we report on surface-optical modes that originate from the tracklike superstructure of the nanorod assemblies.

  2. Optical phonon lasing and its detection in transport through semiconduc- tor double quantum dots

    NASA Astrophysics Data System (ADS)

    Okuyama, Rin; Eto, Mikio; Brandes, Tobias

    2014-03-01

    We theoretically propose optical phonon lasing for a double quantum dot (DQD) fabricated in a semiconductor substrate. No additional cavity or resonator is required. We show that the DQD couples to only two phonon modes that act as a natural cavity. The pumping to the upper level is realized by an electric current through the DQD under a finite bias. Using the rate equation in the Born-Markov-Secular approximation, we analyze the enhanced phonon emission when the level spacing in the DQD is tuned to the phonon energy. We find the phonon lasing when the pumping rate is much larger than the phonon decay rate, whereas anti-bunching of phonon emission is observed when the pumping rate is smaller.[1] Our theory can be also applicable to DQDs embedded in nanomechanical resonators to control the vibrating modes. We discuss detection of amplified modes using the electric current and its noise through the DQD, and another DQD fabricated nearby.

  3. Infrared-phonon-polariton resonance of the nonlinear susceptibility in GaAs.

    PubMed

    Dekorsy, T; Yakovlev, V A; Seidel, W; Helm, M; Keilmann, F

    2003-02-01

    Nonlinear probing of the fundamental lattice vibration of polar crystals is shown to reveal insight into higher-order cohesive lattice forces. With a free-electron laser tunable in the far infrared we experimentally investigate the dispersion of the second-order susceptibility due to the phonon resonance in GaAs. We observe a strong resonance enhancement of second harmonic light generation at half the optical phonon frequency, and in addition a minimum at a higher frequency below the phonon frequency. Measuring this frequency and comparison to a theoretical model allows the determination of competing higher-order lattice forces. PMID:12633374

  4. Influence of the optical-acoustic phonon hybridization on phonon scattering and thermal conductivity

    NASA Astrophysics Data System (ADS)

    Li, Wu; Carrete, Jesús; Madsen, Georg K. H.; Mingo, Natalio

    2016-05-01

    We predict a marked effect of optical-acoustic phonon hybridization on phonon scattering and lattice thermal conductivity (κ ), and illustrate it in the case of Fe2Ge3 . This material presents very low-lying optical phonons with an energy of 1.8 meV at the Brillouin zone center, which show avoided crossings with longitudinal acoustic (LA) phonons, due to optical-acoustic phonon polarization hybridization. Because the optical phonons have nonvanishing scattering rates, even a small amount of hybridization with the optical phonon can increase the scattering rates of LA phonons by much more than one order of magnitude, causing the contribution of these phonons to κ to vanish. At low temperatures, the contributions of all LA phonons are eliminated, and thus the avoided crossing leads to a reduction of thermal conductivity by more than half. The scattering rates are very sensitive to the optical-acoustic phonon hybridization strength, characterized by the gap at the avoided crossing point and varied with the wave-vector direction. Our work presents a different reduction mechanism of κ in systems with optical-acoustic phonon hybridization, which can benefit the search for new thermoelectric materials.

  5. Phonovoltaic. I. Harvesting hot optical phonons in a nanoscale p -n junction

    NASA Astrophysics Data System (ADS)

    Melnick, Corey; Kaviany, Massoud

    2016-03-01

    The phonovoltaic (pV) cell is similar to the photovoltaic. It harvests nonequilibrium (hot) optical phonons (Ep ,O) more energetic than the band gap (Δ Ee ,g) to generate power in a p-n junction. We examine the theoretical electron-phonon and phonon-phonon scattering rates, the Boltzmann transport of electrons, and the diode equation and hydrodynamic simulations to describe the operation of a pV cell and develop an analytic model predicting its efficiency. Our findings indicate that a pV material with Ep ,O≃Δ Ee ,g≫kBT , where kBT is the thermal energy, and a strong interband electron-phonon coupling surpasses the thermoelectric limit, provided the optical phonon population is excited in a nanoscale cell, enabling the ensuing local nonequilibrium. Finding and tuning a material with these properties is challenging. In Paper II [C. Melnick and M. Kaviany, Phys. Rev. B 93, 125203 (2016), 10.1103/PhysRevB.93.125203], we tune the band gap of graphite within density functional theory through hydrogenation and the application of isotropic strains. The band gap is tuned to resonate with its energetic optical phonon modes and calculate the ab initio electron-phonon and phonon-phonon scattering rates. While hydrogenation degrades the strong electron-phonon coupling in graphene such that the figure of merit vanishes, we outline the methodology for a continued material search.

  6. High Resolution Phonon-assisted Quasi-resonance Fluorescence Spectroscopy.

    PubMed

    Czarnocki, Cyprian; Kerfoot, Mark L; Casara, Joshua; Jacobs, Andrew R; Jennings, Cameron; Scheibner, Michael

    2016-01-01

    High resolution optical spectroscopy methods are demanding in terms of either technology, equipment, complexity, time or a combination of these. Here we demonstrate an optical spectroscopy method that is capable of resolving spectral features beyond that of the spin fine structure and homogeneous linewidth of single quantum dots (QDs) using a standard, easy-to-use spectrometer setup. This method incorporates both laser and photoluminescence spectroscopy, combining the advantage of laser line-width limited resolution with multi-channel photoluminescence detection. Such a scheme allows for considerable improvement of resolution over that of a common single-stage spectrometer. The method uses phonons to assist in the measurement of the photoluminescence of a single quantum dot after resonant excitation of its ground state transition. The phonon's energy difference allows one to separate and filter out the laser light exciting the quantum dot. An advantageous feature of this method is its straight forward integration into standard spectroscopy setups, which are accessible to most researchers. PMID:27405015

  7. Influence of coherent optical phonon on ultrafast energy relaxation

    NASA Astrophysics Data System (ADS)

    Wang, J. L.; Guo, L.; Liu, C. H.; Xu, X.; Chen, Y. F.

    2015-08-01

    Ultrafast energy relaxation process in Bi2Te3 thin films is studied using a collinear two color pump-probe technique. The coherent optical phonon is enhanced and destroyed by changing the separation times of double pump pulses. The non-oscillatory component of the reflectivity trace after the second pump pulse shows a distinct difference with and without the presence of coherent optical phonons, thus providing a direct evidence of the effect of optical phonon on the hot carrier relaxation process. The deduced characteristic times are systematically smaller when coherent optical phonons are involved in the energy transfer process. Comparatively, the conventional relaxation process is relatively slow, which is explained by the screening effect of the incoherent optical phonon. This work suggests that the energy relaxation can be manipulated through the excitation of coherent optical phonons.

  8. Phonon Properties of Materials from Neutron Resonance Doppler Broadening Measurements

    NASA Astrophysics Data System (ADS)

    Eric Lynn, J.

    2002-12-01

    At low temperatures the Doppler broadened widths of neutron resonances are strongly affected by the phonon characteristics of the material used for making the cross-section measurement. The Doppler width can be expressed in terms of the moments of the phonon spectrum carried by the atomic species with the resonant cross-section. Cross-section measurements made with tungsten and tantalum metals are reviewed here and compared with phonon information obtained by other methods. Applications of the method to a plutonium-gallium alloy and to some lanthanum barium cuprates are described briefly. We discuss possible extensions of the technique and how an epithermal flight path at the SNS may be advantageous.

  9. Raman spectroscopy of magneto-phonon resonances in graphene and graphite

    NASA Astrophysics Data System (ADS)

    Goler, Sarah; Yan, Jun; Pellegrini, Vittorio; Pinczuk, Aron

    2012-08-01

    The magneto-phonon resonance or MPR occurs in semiconductor materials when the energy spacing between Landau levels is continuously tuned to cross the energy of an optical phonon mode. MPRs have been largely explored in bulk semiconductors, in two-dimensional systems and in quantum dots. Recently there has been significant interest in the MPR interactions of the Dirac fermion magneto-excitons in graphene, and a rich splitting and anti-crossing phenomena of the even parity E2g long wavelength optical phonon mode have been theoretically proposed and experimentally observed. The MPR has been found to crucially depend on disorder in the graphene layer. This is a feature that creates new venues for the study of interplays between disorder and interactions in the atomic layers. We review here the fundamentals of MRP in graphene and the experimental Raman scattering works that have led to the observation of these phenomena in graphene and graphite.

  10. Towards phonon photonics: scattering-type near-field optical microscopy reveals phonon-enhanced near-field interaction.

    PubMed

    Hillenbrand, Rainer

    2004-08-01

    Diffraction limits the spatial resolution in classical microscopy or the dimensions of optical circuits to about half the illumination wavelength. Scanning near-field microscopy can overcome this limitation by exploiting the evanescent near fields existing close to any illuminated object. We use a scattering-type near-field optical microscope (s-SNOM) that uses the illuminated metal tip of an atomic force microscope (AFM) to act as scattering near-field probe. The presented images are direct evidence that the s-SNOM enables optical imaging at a spatial resolution on a 10nm scale, independent of the wavelength used (lambda=633 nm and 10 microm). Operating the microscope at specific mid-infrared frequencies we found a tip-induced phonon-polariton resonance on flat polar crystals such as SiC and Si3N4. Being a spectral fingerprint of any polar material such phonon-enhanced near-field interaction has enormous applicability in nondestructive, material-specific infrared microscopy at nanoscale resolution. The potential of s-SNOM to study eigenfields of surface polaritons in nanostructures opens the door to the development of phonon photonics-a proposed infrared nanotechnology that uses localized or propagating surface phonon polaritons for probing, manipulating and guiding infrared light in nanoscale devices, analogous to plasmon photonics. PMID:15231334

  11. Unified theory of electron-phonon renormalization and phonon-assisted optical absorption

    NASA Astrophysics Data System (ADS)

    Patrick, Christopher E.; Giustino, Feliciano

    2014-09-01

    We present a theory of electronic excitation energies and optical absorption spectra which incorporates energy-level renormalization and phonon-assisted optical absorption within a unified framework. Using time-independent perturbation theory we show how the standard approaches for studying vibronic effects in molecules and those for addressing electron-phonon interactions in solids correspond to slightly different choices for the non-interacting Hamiltonian. Our present approach naturally leads to the Allen-Heine theory of temperature-dependent energy levels, the Franck-Condon principle, the Herzberg-Teller effect and to phonon-assisted optical absorption in indirect band gap materials. In addition, our theory predicts sub-gap phonon-assisted optical absorption in direct gap materials, as well as an exponential edge which we tentatively assign to the Urbach tail. We also consider a semiclassical approach to the calculation of optical absorption spectra which simultaneously captures energy-level renormalization and phonon-assisted transitions and is especially suited to first-principles electronic structure calculations. We demonstrate this approach by calculating the phonon-assisted optical absorption spectrum of bulk silicon.

  12. Determination of phonon decay rate in p-type silicon under Fano resonance by measurement of coherent phonons

    NASA Astrophysics Data System (ADS)

    Kato, Keiko; Oguri, Katsuya; Sanada, Haruki; Tawara, Takehiko; Sogawa, Tetsuomi; Gotoh, Hideki

    2015-09-01

    We determine phonon decay rate by measuring the temperature dependence of coherent phonons in p-type Si under Fano resonance, where there is interference between the continuum and discrete states. As the temperature decreases, the decay rate of coherent phonons decreases, whereas that evaluated from the Raman linewidth increases. The former follows the anharmonic decay model, whereas the latter does not. The different temperature dependences of the phonon decay rate of the two methods originate from the way that the continuum state, which originates from the Fano resonance, modifies the time- and frequency-domain spectra. The observation of coherent phonons is useful for evaluating the phonon decay rate free from the interaction with the continuum state and clarifies that the anharmonic decay is dominant in p-type Si even under Fano resonance.

  13. Raman spectroscopic investigation of the confined optical phonon modes in the aligned CdSe nanorod arrays

    NASA Astrophysics Data System (ADS)

    Nobile, Concetta; Carbone, Luigi; Kudera, Stefan; Manna, Liberato; Cingolani, Roberto; Krahne, Roman; Fonoberov, Vladimir A.; Balandin, Alexander A.; Chilla, Gerwin; Kipp, Tobias; Heitmann, Detlef

    2007-03-01

    Nanocrystal rods have emerged as promising nanostructured material for both fundamental studies of nanoscale effects and for optical and electronic device applications. We investigated the optical phonon excitations in laterally aligned CdSe nanocrystal rod arrays using resonant Raman scattering. Electric-field mediated alignment between interdigitated electrodes has been used to prepare the samples. We report Raman experiments that probe the optical lattice vibrations in ordered arrays of CdSe nanorods with respect to the nanorod orientation. The packing of nanorods into dense arrays leads to the suppression of the surface optical phonon modes. In the longitudinal-optical phonon peak we observe a fine structure that depends on the relative orientation of the nanorods with respect to the incident light polarization. Detailed comparison of the experimental data with the first-principle calculations for corresponding nanostructures, which reveal the symmetry of the phonon potentials for the Raman active modes, provides a qualitative explanation of the experimentally observed phonon modes.

  14. Phonon-assisted exciton transfer into silicon using nanoemitters: the role of phonons and temperature effects in Förster resonance energy transfer.

    PubMed

    Yeltik, Aydan; Guzelturk, Burak; Hernandez-Martinez, Pedro Ludwig; Govorov, Alexander O; Demir, Hilmi Volkan

    2013-12-23

    We study phonon-assisted Förster resonance energy transfer (FRET) into an indirect band-gap semiconductor using nanoemitters. The unusual temperature dependence of this energy transfer, which is measured using the donor nanoemitters of quantum dot (QD) layers integrated on the acceptor monocrystalline bulk silicon as a model system, is predicted by a phonon-assisted exciton transfer model proposed here. The model includes the phonon-mediated optical properties of silicon, while considering the contribution from the multimonolayer-equivalent QD film to the nonradiative energy transfer, which is derived with a d(-3) distance dependence. The FRET efficiencies are experimentally observed to decrease at cryogenic temperatures, which are well explained by the model considering the phonon depopulation in the indirect band-gap acceptor together with the changes in the quantum yield of the donor. These understandings will be crucial for designing FRET-enabled sensitization of silicon based high-efficiency excitonic systems using nanoemitters. PMID:24274734

  15. Sapphire surface polariton splitting due to resonance with aluminum nitride film phonon

    NASA Astrophysics Data System (ADS)

    Yakovlev, V. A.; Novikova, N. N.; Vinogradov, E. A.; Ng, S. S.; Hassan, Z.; Hassan, H. A.

    2010-02-01

    Two thin aluminum nitride films have been prepared on sapphire substrates by molecular beam epitaxy technique. Then alkaline and acidic washing were used to remove the back-metal-coating of the sapphire substrate for one of the samples. (It caused also partial film dissolution). The surface polariton (SP) spectra have been measured by attenuated total reflection (ATR) technique. The measured SP dispersion is compared with one calculated using the literature film parameters. Due to the resonance interaction of sapphire substrate SP with the film transverse optical (TO) phonon the splitting of the dispersion curve of sapphire SP was found. The resonance takes place only for the frequency of the film TO phonon polarized along the surface of the anisotropic AlN film (perpendicular to the optical axis). The analysis of ATR and external reflectivity spectra shows the presence of some transition layer between the substrate and the film.

  16. Mode- and Direction-Dependent Mechanical Energy Dissipation in Single-Crystal Resonators due to Anharmonic Phonon-Phonon Scattering

    NASA Astrophysics Data System (ADS)

    Iyer, Srikanth S.; Candler, Robert N.

    2016-03-01

    In this work, we determine the intrinsic mechanical energy dissipation limit for single-crystal resonators due to anharmonic phonon-phonon scattering in the Akhiezer (Ω τ ≪1 ) regime. The energy loss is derived using perturbation theory and the linearized Boltzmann transport equation for phonons, and includes the direction- and polarization-dependent mode-Grüneisen parameters in order to capture the strain-induced anharmonicity among phonon branches. This expression reveals the fundamental differences among the internal friction limits for different types of bulk-mode elastic waves. For cubic crystals, 2D-extensional modes have increased dissipation compared to width-extensional modes because the biaxial deformation opposes the natural Poisson contraction of the solid. Additionally, we show that shear-mode vibrations, which preserve volume, have significantly reduced energy loss because dissipative phonon-phonon scattering is restricted to pure-shear phonon branches, indicating that Lamé- or wineglass-mode resonators will have the highest upper limit on mechanical efficiency. Finally, we employ key simplifications to evaluate the quality factor limits for common mode shapes in single-crystal silicon devices, explicitly including the correct effective elastic storage moduli for different vibration modes and crystal orientations. Our expression satisfies the pressing need for a reliable analytical model that can predict the phonon-phonon dissipation limits for modern resonant microelectromechanical systems, where precise manufacturing techniques and accurate finite-element methods can be used to select particular vibrational mode shapes and crystal orientations.

  17. Coherent phonon optics in a chip with an electrically controlled active device

    PubMed Central

    Poyser, Caroline L.; Akimov, Andrey V.; Campion, Richard P.; Kent, Anthony J.

    2015-01-01

    Phonon optics concerns operations with high-frequency acoustic waves in solid media in a similar way to how traditional optics operates with the light beams (i.e. photons). Phonon optics experiments with coherent terahertz and sub-terahertz phonons promise a revolution in various technical applications related to high-frequency acoustics, imaging, and heat transport. Previously, phonon optics used passive methods for manipulations with propagating phonon beams that did not enable their external control. Here we fabricate a phononic chip, which includes a generator of coherent monochromatic phonons with frequency 378 GHz, a sensitive coherent phonon detector, and an active layer: a doped semiconductor superlattice, with electrical contacts, inserted into the phonon propagation path. In the experiments, we demonstrate the modulation of the coherent phonon flux by an external electrical bias applied to the active layer. Phonon optics using external control broadens the spectrum of prospective applications of phononics on the nanometer scale. PMID:25652241

  18. Long-range interatomic forces can minimize heat transfer: From slowdown of longitudinal optical phonons to thermal conductivity minimum

    NASA Astrophysics Data System (ADS)

    Han, Haoxue; Feng, Lei; Xiong, Shiyun; Shiga, Takuma; Shiomi, Junichiro; Volz, Sebastian; Kosevich, Yuriy A.

    2016-08-01

    We investigate the role of interatomic forces beyond the nearest neighbors on the thermal transport through an atomic junction with a heavy isotope impurity and in a silicon-germanium-like alloy with atomistic calculations. The thermal conductance of the junction incorporating second-nearest-neighbors forces reaches its minimum when the longitudinal optical phonon resonances in the phonon transmission are minimized. We relate the weakening of the optical phonon resonance with the flattening of the longitudinal optical phonon band of the infinite diatomic lattice with second-nearest-neighbors forces, which is the limit of an extended junction. We emphasize that the bypass of the heavy-atom components in the diatomic lattice by long-range interatomic bonds is crucial for the realization of the minimum in bulk thermal conductivity. We highlight the connection between the minimal thermal conductivity of a SiGe-like alloy with the flattening of the longitudinal optical phonon band of the diatomic lattice due to the second-nearest-neighbors forces, in combination with enhanced anharmonic phonon processes and phonon localizations.

  19. Investigation of anti-Stokes Raman processes at phonon-polariton resonance: from Raman oscillation, frequency upconversion to Raman amplification.

    PubMed

    Ding, Yujie J

    2015-03-01

    Raman oscillation, frequency upconversion, and Raman amplification can be achieved in a second-order nonlinear medium at the phonon-polariton resonance. By beating two optical fields, a second-order nonlinear polarization is generated inside the medium. Such a polarization induces a spatially uniform nonpropagating electric field at the beat frequency, which in turn mixes with the input optical field at the lower frequency to generate or amplify the anti-Stokes optical field. Raman oscillation can be efficiently reached for the copropagating configuration. In comparison, efficient frequency upconversion and large amplifications are achievable for the counterpropagating configuration. These Raman processes can be used to effectively remove transverse-optical phonons before decaying to lower-frequency phonons, achieve laser cooling, and significantly enhance coherent anti-Stokes Raman scattering. The counterpropagating configuration offers advantages for amplifying extremely weak signals. PMID:25723418

  20. Qubit-induced phonon blockade as a signature of quantum behavior in nanomechanical resonators

    SciTech Connect

    Liu Yuxi; Miranowicz, Adam; Gao, Y. B.; Bajer, Jiri; Sun, C. P.; Nori, Franco

    2010-09-15

    The observation of quantized nanomechanical oscillations by detecting femtometer-scale displacements is a significant challenge for experimentalists. We propose that a phonon blockade can serve as a signature of quantum behavior in nanomechanical resonators. In analogy to the photon blockade and Coulomb blockade for electrons, the main idea for phonon blockade is that the second phonon cannot be excited when there is one phonon in the nonlinear oscillator. To realize phonon blockade, a superconducting quantum two-level system is coupled to the nanomechanical resonator and is used to induce the phonon self-interaction. Using Monte Carlo simulations, the dynamics of the induced nonlinear oscillator is studied via the Cahill-Glauber s-parametrized quasiprobability distributions. We show how the oscillation of the resonator can occur in the quantum regime and demonstrate how the phonon blockade can be observed with the currently accessible experimental parameters.

  1. Phonons, defects and optical damage in crystalline acetanilide

    NASA Astrophysics Data System (ADS)

    Kosic, Thomas J.; Hill, Jeffrey R.; Dlott, Dana D.

    1986-04-01

    Intense picosecond pulses cause accumulated optical damage in acetanilide crystals at low temperature. Catastrophic damage to the irradiated volume occurs after an incubation period where defects accumulate. The optical damage is monitored with subanosecond time resolution. The generation of defects is studied with damage-detected picosecond spectroscopy. The accumulation of defects is studied by time-resolved coherent Raman scattering, which is used to measure optical phonon scattering from the accumulating defects.

  2. Unstable optical resonators.

    PubMed

    Kahn, W K

    1966-03-01

    A technique, firmly based on a development from ray optics, is presented for calculating the loss due to the finite sizes of curved mirrors when these form an unstable optical resonator. If paraxial rays launched within such a resonator are confined near the resonator axis, the resonator is termed stable; otherwise it is termed unstable, and is known to have high losses. Siegman has recently presented a geometrical method, brilliantly constructed ad hoc, for calculating these losses in unstable resonators, and indicated where these might be advantageous in laser application. The ray optical theory presented here, which employs the concept of ray modes in an equivalent beam waveguide, is shown to yield results equivalent to those of Siegman for all cases considered by him. However, being derived from conventional ray optics, the validity of the formulas is independently established, and these formulas are immediately applicable to re-entrant resonators and resonators containing inhomogeneous media. The fractional loss per resonator pass is equal to 1-|lambda(2)|, where |lambda(2)| < this 1 is an eigenvalue of the transfer matrix T, representing the corresponding ray transformation. PMID:20048863

  3. Optical phonon modes and crystal structure of NaLaF4 single crystals

    NASA Astrophysics Data System (ADS)

    Lage, Márcio Martins; Matinaga, Franklin Massami; Gesland, Jean-Yves; Moreira, Roberto Luiz

    2006-03-01

    Polarized Raman scattering and infrared reflectivity measurements have been used to investigate the crystal structure of Czochralski-grown NaLaF4 single crystals. The phonon symmetries, the simultaneous presence of polar modes in the infrared and Raman spectra, as well as the observation of piezoelectric resonance, helped us to identify the P6 group as the correct one for this crystal. This material belongs to a family of sodium lanthanide tetrafluorides (NaLnF4) crystals, whose photoluminescence efficiency is comparable to LiYF4. Therefore, NaLaF4 crystals may be important in the development of diode pumped up-conversion solid-state lasers. The number and behavior of the observed optical phonon modes were analyzed in terms of group theory predictions for the group symmetry found. A few anomalies in the phonon characteristics are discussed in terms of cationic disorder in the crystal lattice.

  4. Edge waves and resonances in two-dimensional phononic crystal plates

    SciTech Connect

    Hsu, Jin-Chen Hsu, Chih-Hsun

    2015-05-07

    We present a numerical study on phononic band gaps and resonances occurring at the edge of a semi-infinite two-dimensional (2D) phononic crystal plate. The edge supports localized edge waves coupling to evanescent phononic plate modes that decay exponentially into the semi-infinite phononic crystal plate. The band-gap range and the number of edge-wave eigenmodes can be tailored by tuning the distance between the edge and the semi-infinite 2D phononic lattice. As a result, a phononic band gap for simultaneous edge waves and plate waves is created, and phononic cavities beside the edge can be built to support high-frequency edge resonances. We design an L3 edge cavity and analyze its resonance characteristics. Based on the band gap, high quality factor and strong confinement of resonant edge modes are achieved. The results enable enhanced control over acoustic energy flow in phononic crystal plates, which can be used in designing micro and nanoscale resonant devices and coupling of edge resonances to other types of phononic or photonic crystal cavities.

  5. Low-loss, extreme subdiffraction photon confinement via silicon carbide localized surface phonon polariton resonators.

    PubMed

    Caldwell, Joshua D; Glembocki, Orest J; Francescato, Yan; Sharac, Nicholas; Giannini, Vincenzo; Bezares, Francisco J; Long, James P; Owrutsky, Jeffrey C; Vurgaftman, Igor; Tischler, Joseph G; Wheeler, Virginia D; Bassim, Nabil D; Shirey, Loretta M; Kasica, Richard; Maier, Stefan A

    2013-08-14

    Plasmonics provides great promise for nanophotonic applications. However, the high optical losses inherent in metal-based plasmonic systems have limited progress. Thus, it is critical to identify alternative low-loss materials. One alternative is polar dielectrics that support surface phonon polariton (SPhP) modes, where the confinement of infrared light is aided by optical phonons. Using fabricated 6H-silicon carbide nanopillar antenna arrays, we report on the observation of subdiffraction, localized SPhP resonances. They exhibit a dipolar resonance transverse to the nanopillar axis and a monopolar resonance associated with the longitudinal axis dependent upon the SiC substrate. Both exhibit exceptionally narrow linewidths (7-24 cm(-1)), with quality factors of 40-135, which exceed the theoretical limit of plasmonic systems, with extreme subwavelength confinement of (λ(res)3/V(eff))1/3 = 50-200. Under certain conditions, the modes are Raman-active, enabling their study in the visible spectral range. These observations promise to reinvigorate research in SPhP phenomena and their use for nanophotonic applications. PMID:23815389

  6. Optical phonons in PbTe/CdTe multilayer heterostructures

    SciTech Connect

    Novikova, N. N.; Yakovlev, V. A.; Kucherenko, I. V.; Karczewski, G.; Aleshchenko, Yu. A.; Muratov, A. V.; Zavaritskaya, T. N.; Melnik, N. N.

    2015-05-15

    The infrared reflection spectra of PbTe/CdTe multilayer nanostructures grown by molecular-beam epitaxy are measured in the frequency range of 20–5000 cm{sup −1} at room temperature. The thicknesses and high-frequency dielectric constants of the PbTe and CdTe layers and the frequencies of the transverse optical (TO) phonons in these structures are determined from dispersion analysis of the spectra. It is found that the samples under study are characterized by two TO phonon frequencies, equal to 28 and 47 cm{sup −1}. The first frequency is close to that of TO phonons in bulk PbTe, and the second is assigned to the optical mode in structurally distorted interface layers. The Raman-scattering spectra upon excitation with the radiation of an Ar{sup +} laser at 514.5 nm are measured at room and liquid-nitrogen temperatures. The weak line at 106 cm{sup −1} observed in these spectra is attributed to longitudinal optical phonons in the interface layers.

  7. Resonant enhancement of the zero-phonon emission from a colour centre in a diamond cavity

    NASA Astrophysics Data System (ADS)

    Faraon, Andrei; Barclay, Paul E.; Santori, Charles; Fu, Kai-Mei C.; Beausoleil, Raymond G.

    2011-05-01

    Integrated quantum photonic technologies are key for future applications in quantum information, ultralow-power opto-electronics and sensing. As individual quantum bits, nitrogen-vacancy centres in diamond are among the most promising solid-state systems identified to date, because of their long-lived electron and nuclear spin coherence, and capability for individual optical initialization, readout and information storage. The major outstanding hurdle lies in interconnecting many nitrogen vacancies for large-scale computation. One of the most promising approaches in this regard is to couple them to optical resonators, which can be further interconnected in a photonic network. Here, we demonstrate coupling of the zero-phonon line of individual nitrogen vacancies to the modes of microring resonators fabricated in single-crystal diamond. Zero-phonon line enhancement by more than a factor of 10 is estimated from lifetime measurements. The devices are fabricated using standard semiconductor techniques and off-the-shelf materials, thus enabling integrated diamond photonics.

  8. Coherent phonons excited by two optical pulses

    NASA Astrophysics Data System (ADS)

    Semenov, A. L.; Bezbat'ko, D. N.

    2016-02-01

    Theoretical dependences of the amplitude A and phase φ of photoinduced coherent oscillations of the crystal lattice on the delay time μ between two exciting optical pulses have been derived. It has been shown that φ(μ) is a periodic or decreasing function depending on the experimental conditions. Comparison with the experiment on Bi has been carried out.

  9. Resonant interactions between discrete phonons in quinhydrone driven by nonlinear electron-phonon coupling

    NASA Astrophysics Data System (ADS)

    Rury, Aaron S.

    2016-06-01

    This study reports experimental, computational, and theoretical evidence for a previously unobserved coherent phonon-phonon interaction in an organic solid that can be described by the application of Fano's analysis to a case without the presence of a continuum. Using Raman spectroscopy of the hydrogen-bonded charge-transfer material quinhydrone, two peaks appear near 700 cm-1 we assign as phonons whose position and line-shape asymmetry depend on the sample temperature and light scattering excitation energy. Density functional theory calculations find two nearly degenerate phonons possessing frequencies near the values found in experiment that share similar atomic motion out of the aromatic plane of electron donor and acceptor molecules of quinhydrone. Further analytical modeling of the steady-state light scattering process using the Peierls-Hubbard Hamiltonian and time-dependent perturbation theory motivates assignment of the physical origin of the asymmetric features of each peak's line shape to an interaction between two discrete phonons via nonlinear electron-phonon coupling. In the context of analytical model results, characteristics of the experimental spectra upon 2.33 eV excitation of the Raman scattering process are used to qualify the temperature dependence of the magnitude of this coupling in the valence band of quinhydrone. These results broaden the range of phonon-phonon interactions in materials in general while also highlighting the rich physics and fundamental attributes specific to organic solids that may determine their applicability in next generation electronics and photonics technologies.

  10. Resonant optical gun.

    PubMed

    Maslov, A V; Bakunov, M I

    2014-05-01

    We propose a concept of a structure-a resonant optical gun-to realize an efficient propulsion of dielectric microparticles by light forces. The structure is based on a waveguide in which a reversal of the electromagnetic momentum flow of the incident mode is realized by exciting a whispering gallery resonance in the microparticle. The propelling force can reach the value up to the theoretical maximum of twice the momentum flow of the initial wave. The force density oscillates along the particle periphery and has very large amplitude. PMID:24784113

  11. Interaction of an electron-hole plasma with optical phonons in GaP

    NASA Astrophysics Data System (ADS)

    Smith, G. O.; Juhasz, T.; Bron, W. E.; Levinson, Y. B.

    1992-04-01

    The interaction of an optically induced nonstationary electron-hole plasma with coherently excited optical phonons in GaP has been investigated through time-resolved coherent anti-Stokes Raman spectroscopy. Nonexponential optical-phonon dephasing is observed in the presence of the electron-hole plasma. A model describing the interaction between the optical phonons and the electron-hole plasma is presented. A comparison of results from the theoretical model and from the experimental data indicates good agreement.

  12. Atypical Exciton-Phonon Interactions in WS2 and WSe2 Monolayers Revealed by Resonance Raman Spectroscopy.

    PubMed

    Del Corro, E; Botello-Méndez, A; Gillet, Y; Elias, A L; Terrones, H; Feng, S; Fantini, C; Rhodes, Daniel; Pradhan, N; Balicas, L; Gonze, X; Charlier, J-C; Terrones, M; Pimenta, M A

    2016-04-13

    Resonant Raman spectroscopy is a powerful tool for providing information about excitons and exciton-phonon coupling in two-dimensional materials. We present here resonant Raman experiments of single-layered WS2 and WSe2 using more than 25 laser lines. The Raman excitation profiles of both materials show unexpected differences. All Raman features of WS2 monolayers are enhanced by the first-optical excitations (with an asymmetric response for the spin-orbit related XA and XB excitons), whereas Raman bands of WSe2 are not enhanced at XA/B energies. Such an intriguing phenomenon is addressed by DFT calculations and by solving the Bethe-Salpeter equation. These two materials are very similar. They prefer the same crystal arrangement, and their electronic structure is akin, with comparable spin-orbit coupling. However, we reveal that WS2 and WSe2 exhibit quite different exciton-phonon interactions. In this sense, we demonstrate that the interaction between XC and XA excitons with phonons explains the different Raman responses of WS2 and WSe2, and the absence of Raman enhancement for the WSe2 modes at XA/B energies. These results reveal unusual exciton-phonon interactions and open new avenues for understanding the two-dimensional materials physics, where weak interactions play a key role coupling different degrees of freedom (spin, optic, and electronic). PMID:26998817

  13. A model for longitudinal optical phonons and electron-phonon coupling in GaAs/GaAlAs multilayer structure

    NASA Astrophysics Data System (ADS)

    Guillemot, C.; Clerot, F.

    A new model for long-wavelength longitudinal optical phonons in GaAsGaAlAs multi-layer structures is presented. Depending on the layer, the relative ionic displacements are written on the basis of GaAs or GaAs-type longitudinal optical phonons and treated in the framework of the Born-Huang model generalized to include isotropic dispersion effects in the Brillouin zone centre. For double heterostructures, a finite number of quantized confined modes is found. Interplay between the long range Coulomb interaction, which couples the vibrations of adjacent GaAs layers, and confinement effects, which prevent the displacements of adjacent GaAs layers to overlap, is evidenced in the case of superlattices. The strength of the electron-phonon coupling in double heterostructures stays within a factor of 2 of the electron-bulk phonon effective coupling strength for practical values of the parameters.

  14. Phonon-assisted nonlinear optical processes in ultrashort-pulse pumped optical parametric amplifiers

    NASA Astrophysics Data System (ADS)

    Isaienko, Oleksandr; Robel, István

    2016-03-01

    Optically active phonon modes in ferroelectrics such as potassium titanyl phosphate (KTP) and potassium titanyl arsenate (KTA) in the ~7–20 THz range play an important role in applications of these materials in Raman lasing and terahertz wave generation. Previous studies with picosecond pulse excitation demonstrated that the interaction of pump pulses with phonons can lead to efficient stimulated Raman scattering (SRS) accompanying optical parametric oscillation or amplification processes (OPO/OPA), and to efficient polariton-phonon scattering. In this work, we investigate the behavior of infrared OPAs employing KTP or KTA crystals when pumped with ~800-nm ultrashort pulses of duration comparable to the oscillation period of the optical phonons. We demonstrate that under conditions of coherent impulsive Raman excitation of the phonons, when the effective χ(2) nonlinearity cannot be considered instantaneous, the parametrically amplified waves (most notably, signal) undergo significant spectral modulations leading to an overall redshift of the OPA output. The pump intensity dependence of the redshifted OPA output, the temporal evolution of the parametric gain, as well as the pump spectral modulations suggest the presence of coupling between the nonlinear optical polarizations PNL of the impulsively excited phonons and those of parametrically amplified waves.

  15. Phonon-assisted nonlinear optical processes in ultrashort-pulse pumped optical parametric amplifiers

    PubMed Central

    Isaienko, Oleksandr; Robel, István

    2016-01-01

    Optically active phonon modes in ferroelectrics such as potassium titanyl phosphate (KTP) and potassium titanyl arsenate (KTA) in the ~7–20 THz range play an important role in applications of these materials in Raman lasing and terahertz wave generation. Previous studies with picosecond pulse excitation demonstrated that the interaction of pump pulses with phonons can lead to efficient stimulated Raman scattering (SRS) accompanying optical parametric oscillation or amplification processes (OPO/OPA), and to efficient polariton-phonon scattering. In this work, we investigate the behavior of infrared OPAs employing KTP or KTA crystals when pumped with ~800-nm ultrashort pulses of duration comparable to the oscillation period of the optical phonons. We demonstrate that under conditions of coherent impulsive Raman excitation of the phonons, when the effective χ(2) nonlinearity cannot be considered instantaneous, the parametrically amplified waves (most notably, signal) undergo significant spectral modulations leading to an overall redshift of the OPA output. The pump intensity dependence of the redshifted OPA output, the temporal evolution of the parametric gain, as well as the pump spectral modulations suggest the presence of coupling between the nonlinear optical polarizations PNL of the impulsively excited phonons and those of parametrically amplified waves. PMID:26975881

  16. Phonon-assisted nonlinear optical processes in ultrashort-pulse pumped optical parametric amplifiers

    DOE PAGESBeta

    Isaienko, Oleksandr; Robel, Istvan

    2016-03-15

    Optically active phonon modes in ferroelectrics such as potassium titanyl phosphate (KTP) and potassium titanyl arsenate (KTA) in the ~7–20 THz range play an important role in applications of these materials in Raman lasing and terahertz wave generation. Previous studies with picosecond pulse excitation demonstrated that the interaction of pump pulses with phonons can lead to efficient stimulated Raman scattering (SRS) accompanying optical parametric oscillation or amplification processes (OPO/OPA), and to efficient polariton-phonon scattering. In this work, we investigate the behavior of infrared OPAs employing KTP or KTA crystals when pumped with ~800-nm ultrashort pulses of duration comparable to themore » oscillation period of the optical phonons. We demonstrate that under conditions of coherent impulsive Raman excitation of the phonons, when the effective χ(2) nonlinearity cannot be considered instantaneous, the parametrically amplified waves (most notably, signal) undergo significant spectral modulations leading to an overall redshift of the OPA output. Furthermore, the pump intensity dependence of the redshifted OPA output, the temporal evolution of the parametric gain, as well as the pump spectral modulations suggest the presence of coupling between the nonlinear optical polarizations PNL of the impulsively excited phonons and those of parametrically amplified waves.« less

  17. Phonon-assisted nonlinear optical processes in ultrashort-pulse pumped optical parametric amplifiers.

    PubMed

    Isaienko, Oleksandr; Robel, István

    2016-01-01

    Optically active phonon modes in ferroelectrics such as potassium titanyl phosphate (KTP) and potassium titanyl arsenate (KTA) in the ~7-20 THz range play an important role in applications of these materials in Raman lasing and terahertz wave generation. Previous studies with picosecond pulse excitation demonstrated that the interaction of pump pulses with phonons can lead to efficient stimulated Raman scattering (SRS) accompanying optical parametric oscillation or amplification processes (OPO/OPA), and to efficient polariton-phonon scattering. In this work, we investigate the behavior of infrared OPAs employing KTP or KTA crystals when pumped with ~800-nm ultrashort pulses of duration comparable to the oscillation period of the optical phonons. We demonstrate that under conditions of coherent impulsive Raman excitation of the phonons, when the effective χ((2)) nonlinearity cannot be considered instantaneous, the parametrically amplified waves (most notably, signal) undergo significant spectral modulations leading to an overall redshift of the OPA output. The pump intensity dependence of the redshifted OPA output, the temporal evolution of the parametric gain, as well as the pump spectral modulations suggest the presence of coupling between the nonlinear optical polarizations P(NL) of the impulsively excited phonons and those of parametrically amplified waves. PMID:26975881

  18. Aspect-ratio driven evolution of high-order resonant modes and near-field distributions in localized surface phonon polariton nanostructures.

    PubMed

    Ellis, Chase T; Tischler, Joseph G; Glembocki, Orest J; Bezares, Francisco J; Giles, Alexander J; Kasica, Richard; Shirey, Loretta; Owrutsky, Jeffrey C; Chigrin, Dmitry N; Caldwell, Joshua D

    2016-01-01

    Polar dielectrics have garnered much attention as an alternative to plasmonic metals in the mid- to long-wave infrared spectral regime due to their low optical losses. As such, nanoscale resonators composed of these materials demonstrate figures of merit beyond those achievable in plasmonic equivalents. However, until now, only low-order, phonon-mediated, localized polariton resonances, known as surface phonon polaritons (SPhPs), have been observed in polar dielectric optical resonators. In the present work, we investigate the excitation of 16 distinct high-order, multipolar, localized surface phonon polariton resonances that are optically excited in rectangular pillars etched into a semi-insulating silicon carbide substrate. By elongating a single pillar axis we are able to significantly modify the far- and near-field properties of localized SPhP resonances, opening the door to realizing narrow-band infrared sources with tailored radiation patterns. Such control of the near-field behavior of resonances can also impact surface enhanced infrared optical sensing, which is mediated by polarization selection rules, as well as the morphology and strength of resonator hot spots. Furthermore, through the careful choice of polar dielectric material, these results can also serve as the guiding principles for the generalized design of optical devices that operate from the mid- to far-infrared. PMID:27622525

  19. Reducing support loss in micromechanical ring resonators using phononic band-gap structures

    NASA Astrophysics Data System (ADS)

    Hsu, Feng-Chia; Hsu, Jin-Chen; Huang, Tsun-Che; Wang, Chin-Hung; Chang, Pin

    2011-09-01

    In micromechanical resonators, energy loss via supports into the substrates may lead to a low quality factor. To eliminate the support loss, in this paper a phononic band-gap structure is employed. We demonstrate a design of phononic-crystal (PC) strips used to support extensional wine-glass mode ring resonators to increase the quality factor. The PC strips are introduced to stop elastic-wave propagation by the band-gap and deaf-band effects. Analyses of resonant characteristics of the ring resonators and the dispersion relations, eigenmodes, and transmission properties of the PC strips are presented. With the proposed resonator architecture, the finite-element simulations show that the leaky power is effectively reduced and the stored energy inside the resonators is enhanced simultaneously as the operating frequencies of the resonators are within the band gap or deaf bands. Realization of a high quality factor micromechanical ring resonator with minimized support loss is expected.

  20. Semiconductor superlattice diodes for detection of terahertz photons: The role of hybridization of the plasma and polar-optical phonon modes

    SciTech Connect

    Ignatov, Anatoly A.

    2014-08-28

    The current (voltage) responsivity of a superlattice-based diode detector has been studied theoretically in the terahertz frequency band that includes the region of the polar-optical phonon frequencies. Within the framework of an equivalent circuit approach, the electro-dynamical model which allows one to analyze the responsivity taking into account the hybridization of the plasma and polar-optical phonon modes both in the substrate and in the cladding layers of the diode has been suggested. It has been shown that the presence of the plasma and polar-optical phonon modes gives rise to strong features in the frequency dependence of the responsivity, i.e., to the resonance dips and peaks at frequencies of hybridized plasmons and polar-optical phonons. It has been suggested that by judicious engineering of the superlattice-based diodes, it would be possible to enhance substantially their responsivity in the terahertz frequency band.

  1. Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals

    PubMed Central

    He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-hu; Xiao, Min

    2016-01-01

    A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction. PMID:27457385

  2. Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals

    NASA Astrophysics Data System (ADS)

    He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-Hu; Xiao, Min

    2016-07-01

    A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction.

  3. Coherent optical phonon oscillation and possible electronic softening in WTe2 crystals.

    PubMed

    He, Bin; Zhang, Chunfeng; Zhu, Weida; Li, Yufeng; Liu, Shenghua; Zhu, Xiyu; Wu, Xuewei; Wang, Xiaoyong; Wen, Hai-Hu; Xiao, Min

    2016-01-01

    A rapidly-growing interest in WTe2 has been triggered by the giant magnetoresistance effect discovered in this unique system. While many efforts have been made towards uncovering the electron- and spin-relevant mechanisms, the role of lattice vibration remains poorly understood. Here, we study the coherent vibrational dynamics in WTe2 crystals by using ultrafast pump-probe spectroscopy. The oscillation signal in time domain in WTe2 has been ascribed as due to the coherent dynamics of the lowest energy A1 optical phonons with polarization- and wavelength-dependent measurements. With increasing temperature, the phonon energy decreases due to anharmonic decay of the optical phonons into acoustic phonons. Moreover, a significant drop (15%) of the phonon energy with increasing pump power is observed which is possibly caused by the lattice anharmonicity induced by electronic excitation and phonon-phonon interaction. PMID:27457385

  4. Nonlinear optical whispering gallery mode resonators

    NASA Technical Reports Server (NTRS)

    Ilchenko, Vladimir (Inventor); Matsko, Andrey B. (Inventor); Savchenkov, Anatoliy (Inventor); Maleki, Lutfollah (Inventor)

    2005-01-01

    Whispering gallery mode (WGM) optical resonators comprising nonlinear optical materials, where the nonlinear optical material of a WGM resonator includes a plurality of sectors within the optical resonator and nonlinear coefficients of two adjacent sectors are oppositely poled.

  5. Electron quasi-confined-optical-phonon interactions in wurtzite GaN/AlN quantum wells

    NASA Astrophysics Data System (ADS)

    Li, L.; Liu, D.; Shi, J.-J.

    2005-04-01

    The equation of motion for the p-polarization field in a wurtzite GaN/AlN multilayer heterostructure is solved for the quasi-confined-optical-phonon modes based on the dielectric-continuum model and Loudon’s uniaxial crystal model. The polarization eigenvector, the dispersion relation of the quasi-confined-optical-phonon modes and the electron-quasi-confined-phonon interaction Fröhlich-like Hamiltonian are derived. The analytical formulas can be directly applied to single/multiple quantum wells (QW’s) and superlattices. The electron-quasi-confined-phonon coupling functions are investigated for a given AlN/GaN/AlN single QW with full account of the strains of the QW structures and the anisotropy effect of wurtzite crystals. We find that there are two kinds of quasi-confined-optical-phonon modes in the GaN/AlN QW’s: the GaN-layer quasi-confined-optical-phonon modes and the AlN-layer quasi-confined-optical-phonon modes. There are infinite quasi-confined-optical-phonon branches, labelled by a quantum number n (n=1,2,...), with definite symmetry with respect to the center of the AlN/GaN/AlN single QW for a given phonon wave number q. The dispersions of the quasi-confined-optical-phonon modes with smaller n are more obvious than the ones with larger n. Moreover, the modes with smaller n are much more important for their electron-quasi-confined-phonon interactions than those with larger n. In most cases, it is enough to consider the modes with n≤ 8 for the electron-quasi-confined-phonon interactions in a single GaN/AlN QW. The higher frequency modes are more significant than the lower ones. The long-wavelength quasi-confined-optical-phonon modes are much more important for the electron-quasi-confined-phonon interactions. The GaN-layer quasi-confined-optical-phonon energies and their electron-quasi-confined-phonon interaction strength are markedly increased due to the strains of the QW structures. The influence of the strains on the the AlN-layer electron-quasi-confined-phonon

  6. Effect of stress and temperature on the optical phonons of aramid fibers

    NASA Astrophysics Data System (ADS)

    Bollas, D.; Parthenios, J.; Galiotis, C.

    2006-03-01

    The wave-number dependence upon stress and/or strain and temperature of two adjacent optical phonons of aramid fibers has been investigated. The results showed that both phonons soften considerably under axial tension. Experiments at various temperatures under fixed strain conditions have demonstrated that one of the phonons (ν1=1611cm-1) is moderately anharmonic whereas the adjacent phonon (ν2=1648cm-1) exhibits harmonic behavior. By modeling the fibers as one-dimensional molecular wires very good agreement between experiment and theory is obtained for the phonon temperature dependence under isostress conditions.

  7. Sound and noisy light: Optical control of phonons in photoswitchable structures

    NASA Astrophysics Data System (ADS)

    Sklan, Sophia R.; Grossman, Jeffrey C.

    2015-10-01

    We present a means of controlling phonons via optical tuning. Taking as a model an array of photoresponsive materials (photoswitches) embedded in a matrix, we numerically analyze the vibrational response of an array of bistable harmonic oscillators with stochastic spring constants. Changing the intensity of light incident on the lattice directly controls the composition of the lattice and therefore the speed of sound. Furthermore, modulation of the phonon band structure at high frequencies results in a strong confinement of phonons. The applications of this regime for phonon waveguides, vibrational energy storage, and phononic transistors is examined.

  8. Plasmon-optical phonon hybridization in polar semiconductor nano-wires

    NASA Astrophysics Data System (ADS)

    Moradi, Afshin

    2013-12-01

    The hybridization of the plasmon oscillations with the optical phonon waves in cylindrical polar semiconductor nano-wires is investigated. A simple model based on the hydrodynamic theory in conjunction with the Poisson's equation is proposed. An explicit form of the dispersion relation for hybridized surface plasmon-optical phonon modes of the system is derived.

  9. Raman selection rule for surface optical phonons in ZnS nanobelts.

    PubMed

    Ho, Chih-Hsiang; Varadhan, Purushothaman; Wang, Hsin-Hua; Chen, Cheng-Ying; Fang, Xiaosheng; He, Jr-Hau

    2016-03-21

    We report Raman scattering results for high-quality wurtzite ZnS nanobelts (NBs) grown by chemical vapor deposition. In the Raman spectrum, the ensembles of ZnS NBs exhibit first order phonon modes at 274 cm(-1) and 350 cm(-1), corresponding to A1/E1 transverse optical and A1/E1 longitudinal optical phonons, in addition to a strong surface optical (SO) phonon mode at 329 cm(-1). The existence of the SO band is confirmed by its shift with different surrounding dielectric media. Polarization dependent Raman spectra were recorded on a single ZnS NB and for the first time a SO phonon band has been detected on a single nanobelt. Different selection rules for the SO phonon mode are shown from their corresponding E1/A1 phonon modes, and were attributed to the breaking of anisotropic translational symmetry on the NB surface. PMID:26924069

  10. Reversible optical switching of highly confined phonon-polaritons with an ultrathin phase-change material

    NASA Astrophysics Data System (ADS)

    Li, Peining; Yang, Xiaosheng; Maß, Tobias W. W.; Hanss, Julian; Lewin, Martin; Michel, Ann-Katrin U.; Wuttig, Matthias; Taubner, Thomas

    2016-08-01

    Surface phonon-polaritons (SPhPs), collective excitations of photons coupled with phonons in polar crystals, enable strong light-matter interaction and numerous infrared nanophotonic applications. However, as the lattice vibrations are determined by the crystal structure, the dynamical control of SPhPs remains challenging. Here, we realize the all-optical, non-volatile, and reversible switching of SPhPs by controlling the structural phase of a phase-change material (PCM) employed as a switchable dielectric environment. We experimentally demonstrate optical switching of an ultrathin PCM film (down to 7 nm, <λ/1,200) with single laser pulses and detect ultra-confined SPhPs (polariton wavevector kp > 70k0, k0 = 2π/λ) in quartz. Our proof of concept allows the preparation of all-dielectric, rewritable SPhP resonators without the need for complex fabrication methods. With optimized materials and parallelized optical addressing we foresee application potential for switchable infrared nanophotonic elements, for example, imaging elements such as superlenses and hyperlenses, as well as reconfigurable metasurfaces and sensors.

  11. Optimization of a Tunable Piezoelectric Resonator Using Phononic Crystals with Periodic Electrical Boundary Conditions

    NASA Astrophysics Data System (ADS)

    Ponge, Marie-Fraise; Dubus, Bertrand; Granger, Christian; Vasseur, Jérôme; Thi, Mai Pham; Hladky-Hennion, Anne-Christine

    Piezoelectric phononic crystals with periodic short-circuit conditions exhibit Bragg band gaps. They are used to design a Fabry-Perot cavity. The design of the device enables a modification of cavity length by a spatial shift of electrical boundary conditions. The resonator is thus tunable and a frequency shift is obtained. An analytical model based on a transfer matrix formalism is used to model longitudinal wave propagation inside the structure. Cavity length, phononic crystal and transducer position are optimized to increase resonance and antiresonance frequency shifts as well as coupling coefficient. Numerical and experimental results are presented and discussed.

  12. Optical resonator and laser applications

    NASA Technical Reports Server (NTRS)

    Taghavi-Larigani, Shervin (Inventor); Vanzyl, Jakob J. (Inventor); Yariv, Amnon (Inventor)

    2006-01-01

    The invention discloses a semi-ring Fabry-Perot (SRFP) optical resonator structure comprising a medium including an edge forming a reflective facet and a waveguide within the medium, the waveguide having opposing ends formed by the reflective facet. The performance of the SRFP resonator can be further enhanced by including a Mach-Zehnder interferometer in the waveguide on one side of the gain medium. The optical resonator can be employed in a variety of optical devices. Laser structures using at least one SRFP resonator are disclosed where the resonators are disposed on opposite sides of a gain medium. Other laser structures employing one or more resonators on one side of a gain region are also disclosed.

  13. Phonon-Assisted Resonant Tunneling of Electrons in Graphene-Boron Nitride Transistors.

    PubMed

    Vdovin, E E; Mishchenko, A; Greenaway, M T; Zhu, M J; Ghazaryan, D; Misra, A; Cao, Y; Morozov, S V; Makarovsky, O; Fromhold, T M; Patanè, A; Slotman, G J; Katsnelson, M I; Geim, A K; Novoselov, K S; Eaves, L

    2016-05-01

    We observe a series of sharp resonant features in the differential conductance of graphene-hexagonal boron nitride-graphene tunnel transistors over a wide range of bias voltages between 10 and 200 mV. We attribute them to electron tunneling assisted by the emission of phonons of well-defined energy. The bias voltages at which they occur are insensitive to the applied gate voltage and hence independent of the carrier densities in the graphene electrodes, so plasmonic effects can be ruled out. The phonon energies corresponding to the resonances are compared with the lattice dispersion curves of graphene-boron nitride heterostructures and are close to peaks in the single phonon density of states. PMID:27203338

  14. Phonon-Assisted Resonant Tunneling of Electrons in Graphene-Boron Nitride Transistors

    NASA Astrophysics Data System (ADS)

    Vdovin, E. E.; Mishchenko, A.; Greenaway, M. T.; Zhu, M. J.; Ghazaryan, D.; Misra, A.; Cao, Y.; Morozov, S. V.; Makarovsky, O.; Fromhold, T. M.; Patanè, A.; Slotman, G. J.; Katsnelson, M. I.; Geim, A. K.; Novoselov, K. S.; Eaves, L.

    2016-05-01

    We observe a series of sharp resonant features in the differential conductance of graphene-hexagonal boron nitride-graphene tunnel transistors over a wide range of bias voltages between 10 and 200 mV. We attribute them to electron tunneling assisted by the emission of phonons of well-defined energy. The bias voltages at which they occur are insensitive to the applied gate voltage and hence independent of the carrier densities in the graphene electrodes, so plasmonic effects can be ruled out. The phonon energies corresponding to the resonances are compared with the lattice dispersion curves of graphene-boron nitride heterostructures and are close to peaks in the single phonon density of states.

  15. Analysis and experimental realization of locally resonant phononic plates carrying a periodic array of beam-like resonators

    NASA Astrophysics Data System (ADS)

    Xiao, Yong; Wen, Jihong; Huang, Lingzhi; Wen, Xisen

    2014-01-01

    We present theoretical examination and experimental demonstration of locally resonant (LR) phononic plates consisting of a periodic array of beam-like resonators attached to a thin homogeneous plate. Such phononic plates feature unique wave physics due to the coexistence of localized resonance and structural periodicity. We demonstrate that a low-frequency complete band gap for flexural plate waves can be created in the proposed structure owing to the interaction between the localized resonant modes of the beam-like resonators and the flexural wave modes of the host plate. We show that the location and width of the complete band gap can be dramatically tuned by changing the properties of the beam-like resonators. To understand the opening mechanism and evolution behaviour of the complete band gap, some approximate but explicit models are provided and discussed. We further perform experimental measurements of a specimen fabricated by an array of double-stacked aluminum beam-like resonators attached to a thin aluminum plate with 5 cm structure periodicity. The experimental results evidence a complete band gap extending from 465 to 860 Hz, matching well with our theoretical prediction. The LR phononic plates proposed in this work can find potential applications in attenuation of low-frequency mechanical vibrations and insulation of low-frequency audible sound.

  16. High-performance Brillouin spectroscopy of phonons induced by a piezoelectric thin film with a coaxial microwave resonator.

    PubMed

    Sano, Hiroyuki; Yanagitani, Takahiko; Takayanagi, Shinji; Sugimoto, Takeshi; Matsukawa, Mami

    2013-05-01

    To overcome the low accuracy of acoustic velocity measurements based on Brillouin scattering from thermal phonons, we attempted to utilize induced coherent phonons, which cause intense Brillouin scattering. A ZnO piezoelectric film was used to induce gigahertz-range coherent phonons in a silica glass block sample. An evanescent electromagnetic wave leaked from a coaxial resonator was applied into the film to excite phonons. The scattered light obtained using this simple system was much more intense than that obtained from thermal phonons. This technique will improve the accuracy and reduce the measurement time. PMID:23661120

  17. Optical Helmholtz resonators

    NASA Astrophysics Data System (ADS)

    Chevalier, Paul; Bouchon, Patrick; Haïdar, Riad; Pardo, Fabrice

    2014-08-01

    Helmholtz resonators are widely used acoustic components able to select a single frequency. Here, based on an analogy between acoustics and electromagnetism wave equations, we present an electromagnetic 2D Helmholtz resonator made of a metallic slit-box structure. At the resonance, the light is funneled in the λ/800 apertures, and is subsequently absorbed in the cavity. As in acoustics, there is no higher order of resonance, which is an appealing feature for applications such as photodetection or thermal emission. Eventually, we demonstrate that the slit is of capacitive nature while the box behaves inductively. We derive an analytical formula for the resonance wavelength, which does not rely on wave propagation and therefore does not depend on the permittivity of the material filling the box. Besides, in contrast with half-wavelength resonators, the resonance wavelength can be engineered by both the slit aspect ratio and the box area.

  18. Elastic filter based on coupled resonator waveguides in phononic crystal slabs

    NASA Astrophysics Data System (ADS)

    Khelif, Abdelkrim; Mohammadi, Saeed; Eftekhar, Ali; Adibi, Ali; Aoubiza, Boujemaa

    2010-02-01

    In this paper we demonstrate the possibility of forming a new elastic filter structure based on the coupled resonator waveguides in phononic crystal slabs (CRAW) with superior performance over the conventional filters. The structures are made by etching a honeycomb array of holes in a free standing slab. This phononic slab structure exhibits an absolute phononic band gap for all polarizations of guided waves inside the slab including the Lamb and Love waves. We present an analysis of a different family of waveguides in phononic-crystal slabs, and illustrate the considerations that must be applied to achieve single-mode guided bands in these structures. Consequently, an unusual family of selective elastic filters composed of several single resonators that are coupled periodically through evanescent waves is obtained. The elastic energy is localized in the extended defect formed by the collective coupled resonators. The frequencies of the filters are sensitive to the geometrical parameters and to the separation distance between the indiviual resonators. Numerical simulations are performed using the finite element method and considering Zinc-Oxide slab.

  19. Femtosecond optical excitation of coherent acoustic phonons in a piezoelectric p-n junction

    NASA Astrophysics Data System (ADS)

    Wen, Yu-Chieh; Chern, Gia-Wei; Lin, Kung-Hsuan; Yeh, Jeffrey Jarren; Sun, Chi-Kuang

    2011-11-01

    We present a theoretical model for the photogeneration of coherent acoustic phonons in a piezoelectric p-n junction. In our model, the transport of photoexcited carriers is governed by the drift-diffusion equation, whereas the dynamics of acoustic phonons obeys a loaded string equation. Among various mechanisms, the piezoelectric coupling is found to dominate the acoustic-phonon generation process. The waveform of the photogenerated acoustic pulse is strongly influenced by the various dynamics of the photoexcited carriers, especially the picosecond hole drifting. Our calculation also confirms the crucial role of the built-in electric field in the formation of coherent acoustic phonons under optical excitations.

  20. Optical properties of amorphous Ge1- x Se x and Ge1- x- y Se x As y thin films — optical gap bowing and phonon modes

    NASA Astrophysics Data System (ADS)

    Lee, Hosuk; So, Hyeon Seob; Lee, Hosun; Shin, Hae-Young; Yoon, Seokhyun; Ahn, Hyung-Woo; Kim, Su-Dong; Lee, Suyoun; Jeong, Doo-Seok; Cheong, Byung-ki

    2014-06-01

    We investigated the optical properties of Ge1- x Se x and Ge1- x- y Se x As y amorphous films by using spectroscopic ellipsometry and Raman spectroscopy. The dielectric functions and absorption coefficients ( α) of the amorphous films were determined from the measured ellipsometric angles (Ψ,Δ). We obtained the optical gap energies and the Urbach energies from the absorption coefficients and found a strong bowing effect in the optical gap energy of Ge1- x- y Se x As y , where the endpoint binaries were Ge0.50Se0.50 and Ge0.31As0.69. Based on the correlation between the optical gap energies and the Urbach energies, we attributed the large bowing parameter to electronic disorder. Using Raman spectroscopy, we measured the phonon modes and discussed the composition dependence of the phonon peak frequencies and lineshapes in terms of structural units. Based on the composition dependence of the phonons in Ge1- x- y Se x As y , we identified the phonon modes of Ge0.31As0.69. A resonant Raman phenomenon was observed in Ge0.40Se0.60 at a laser excitation of 514 nm (2.41 eV). We verified that this laser energy corresponded to the transition energy of Ge0.40Se0.60 by using the second derivative of the dielectric function of Ge0.40Se0.60.

  1. Ultrafast dynamics of coherent optical phonons in GeTe/Sb2Te3 superlattices: thermal conductivity and coherent control

    NASA Astrophysics Data System (ADS)

    Hase, Muneaki; Tominaga, Junji

    2012-03-01

    We report on the evaluation of lattice thermal conductivity of GeTe/Sb2Te3 superlattice (SL) by using a coherent phonon spectroscopy at various lattice temperatures. The time-resolved transient reflectivity obtained in amorphous and crystalline GeTe/Sb2Te3 SL films exhibits the coherent A1 optical modes at terahertz (THz) frequencies with picoseconds dephasing time. The relaxation time and frequency of the coherent A1 modes are used to compute the lattice thermal conductivity based on the Debye theory, including scattering by grain boundary and point defect, umklapp process, and phonon resonant scattering. The results indicate that the thermal conductivity in the amorphous SL film is less temperature dependent, due to the dominant phonon-defect scattering, while in the crystalline SL it is temperature dependent because of the main contributions from umklapp and phonon resonant scatterings. We argue the higher thermal conductivity in the GeTe/Sb2Te3 SL films than that in the Ge2Sb2Te5 alloy films implies that the phase change in GeTe/Sb2Te3 SL is not purely promoted by thermal process, i.e., lattice heating, but rather by nonthermal process, i.e., coherent lattice excitation, because the thermal process generally requires lower thermal conductivity.

  2. Planar modes free piezoelectric resonators using a phononic crystal with holes.

    PubMed

    Aragón, J L; Quintero-Torres, R; Domínguez-Juárez, J L; Iglesias, E; Ronda, S; Montero de Espinosa, F

    2016-09-01

    By using the principles behind phononic crystals, a periodic array of circular holes made along the polarization thickness direction of piezoceramic resonators are used to stop the planar resonances around the thickness mode band. In this way, a piezoceramic resonator adequate for operation in the thickness mode with an in phase vibration surface is obtained, independently of its lateral shape. Laser vibrometry, electric impedance tests and finite element models are used to corroborate the performances of different resonators made with this procedure. This method can be useful in power ultrasonic devices, physiotherapy and other external medical power ultrasound applications where piston-like vibration in a narrow band is required. PMID:27387418

  3. Optical Coherence in Atomic-Monolayer Transition-Metal Dichalcogenides Limited by Electron-Phonon Interactions

    NASA Astrophysics Data System (ADS)

    Dey, P.; Paul, J.; Wang, Z.; Stevens, C. E.; Liu, C.; Romero, A. H.; Shan, J.; Hilton, D. J.; Karaiskaj, D.

    2016-03-01

    We systematically investigate the excitonic dephasing of three representative transition-metal dichalcogenides, namely, MoS2 , MoSe2 , and WSe2 atomic monolayer thick and bulk crystals, in order to gain a proper understanding of the factors that determine the optical coherence in these materials. Coherent nonlinear optical spectroscopy and temperature dependent absorption, combined with theoretical calculations of the phonon spectra, indicate electron-phonon interactions, to be the limiting factor. Surprisingly, the excitonic dephasing, differs only slightly between atomic monolayers and high quality bulk crystals, which indicates that material imperfections are not the limiting factor in atomically thin monolayer samples. The temperature dependence of the electronic band gap and the excitonic linewidth combined with "ab initio" calculations of the phonon energies and the phonon density of states reveal a strong interaction with the E ' and E " phonon modes.

  4. Electron-phonon interaction on optical spectra of nanoelectronic devices

    NASA Technical Reports Server (NTRS)

    Kim, Q.

    2002-01-01

    Information obtained on the solid-state lattice dynamics by electron-phonon interaction between lattice phonons and electrons could open up to learn more about lattice dynamics and to apply it in nanoelectronic devices including software reliability, nano-size capacitors, master clock sources, as well as non-contact temperature probes on nano-electronic and photonicdevices.

  5. Localized surface phonon polariton resonances in polar gallium nitride

    SciTech Connect

    Feng, Kaijun Islam, S. M.; Verma, Jai; Hoffman, Anthony J.; Streyer, William; Wasserman, Daniel; Jena, Debdeep

    2015-08-24

    We demonstrate the excitation of localized surface phonon polaritons in an array of sub-diffraction pucks fabricated in an epitaxial layer of gallium nitride (GaN) on a silicon carbide (SiC) substrate. The array is characterized via polarization- and angle-dependent reflection spectroscopy in the mid-infrared, and coupling to several localized modes is observed in the GaN Reststrahlen band (13.4–18.0 μm). The same structure is simulated using finite element methods and the charge density of the modes are studied; transverse dipole modes are identified for the transverse electric and magnetic polarizations and a quadrupole mode is identified for the transverse magnetic polarization. The measured mid-infrared spectrum agrees well with numerically simulated spectra. This work could enable optoelectronic structures and devices that support surface modes at mid- and far-infrared wavelengths.

  6. Localized surface phonon polariton resonances in polar gallium nitride

    NASA Astrophysics Data System (ADS)

    Feng, Kaijun; Streyer, William; Islam, S. M.; Verma, Jai; Jena, Debdeep; Wasserman, Daniel; Hoffman, Anthony J.

    2015-08-01

    We demonstrate the excitation of localized surface phonon polaritons in an array of sub-diffraction pucks fabricated in an epitaxial layer of gallium nitride (GaN) on a silicon carbide (SiC) substrate. The array is characterized via polarization- and angle-dependent reflection spectroscopy in the mid-infrared, and coupling to several localized modes is observed in the GaN Reststrahlen band (13.4-18.0 μm). The same structure is simulated using finite element methods and the charge density of the modes are studied; transverse dipole modes are identified for the transverse electric and magnetic polarizations and a quadrupole mode is identified for the transverse magnetic polarization. The measured mid-infrared spectrum agrees well with numerically simulated spectra. This work could enable optoelectronic structures and devices that support surface modes at mid- and far-infrared wavelengths.

  7. Phonon-Electron Interactions in Piezoelectric Semiconductor Bulk Acoustic Wave Resonators

    PubMed Central

    Gokhale, Vikrant J.; Rais-Zadeh, Mina

    2014-01-01

    This work presents the first comprehensive investigation of phonon-electron interactions in bulk acoustic standing wave (BAW) resonators made from piezoelectric semiconductor (PS) materials. We show that these interactions constitute a significant energy loss mechanism and can set practical loss limits lower than anharmonic phonon scattering limits or thermoelastic damping limits. Secondly, we theoretically and experimentally demonstrate that phonon-electron interactions, under appropriate conditions, can result in a significant acoustic gain manifested as an improved quality factor (Q). Measurements on GaN resonators are consistent with the presented interaction model and demonstrate up to 35% dynamic improvement in Q. The strong dependencies of electron-mediated acoustic loss/gain on resonance frequency and material properties are investigated. Piezoelectric semiconductors are an extremely important class of electromechanical materials, and this work provides crucial insights for material choice, material properties, and device design to achieve low-loss PS-BAW resonators along with the unprecedented ability to dynamically tune resonator Q. PMID:25001100

  8. Surface polar optical phonon scattering of carriers in graphene on various substrates

    NASA Astrophysics Data System (ADS)

    Lin, I.-Tan; Liu, Jia-Ming

    2013-08-01

    The surface polar optical phonon scattering of carriers in graphene on various substrates is thoroughly studied using Rode's iteration method. The dependence of the scattering rate on carrier energy, temperature, and Fermi energy is investigated. The experimental data in the literature on the temperature dependence of the resistivity can be fitted using only one free fitting parameter. The fitting results show that the coupling strengths of surface optical phonons are much stronger, by at least a factor of 3.5, than the theoretical prediction. The strong coupling also suggests that the deformation potential of acoustic phonons might have been overestimated in the literature.

  9. Phonon coupling in optical transitions for singlet-triplet pairs of bound excitons in semiconductors

    NASA Astrophysics Data System (ADS)

    Pistol, M. E.; Monemar, B.

    1986-05-01

    A model is presented for the observed strong difference in selection rules for coupling of phonons in the one-phonon sideband of optical spectra related to bound excitons in semiconductors. The present treatment is specialized to the case of a closely spaced pair of singlet-triplet character as the lowest electronic states, as is common for bound excitons associated with neutral complexes in materials like GaP and Si. The optical transition for the singlet bound-exciton state is found to couple strongly only to symmetric A1 modes. The triplet state has a similar coupling strength to A1 modes, but in addition strong contributions are found for replicas corresponding to high-density-of-states phonons TAX, LAX, and TOX. This can be explained by a treatment of particle-phonon coupling beyond the ordinary adiabatic approximation. A weak mixing between the singlet and triplet states is mediated by the phonon coupling, as described in first-order perturbation theory. The model derived in this work, for such phonon-induced mixing of closely spaced electronic states, is shown to explain the observed phonon coupling for several bound-exciton systems of singlet-triplet character in GaP. In addition, the observed oscillator strength of the forbidden triplet state may be explained as partly derived from phonon-induced mixing with the singlet state, which has a much larger oscillator strength.

  10. Method for observing robust and tunable phonon blockade in a nanomechanical resonator coupled to a charge qubit

    NASA Astrophysics Data System (ADS)

    Wang, Xin; Miranowicz, Adam; Li, Hong-Rong; Nori, Franco

    2016-06-01

    Phonon blockade is a purely quantum phenomenon, analogous to Coulomb and photon blockades, in which a single phonon in an anharmonic mechanical resonator can impede the excitation of a second phonon. We propose an experimental method to realize phonon blockade in a driven harmonic nanomechanical resonator coupled to a qubit, where the coupling is proportional to the second-order nonlinear susceptibility χ(2 ). This is in contrast to the standard realizations of phonon and photon blockade effects in Kerr-type χ(3 ) nonlinear systems. The nonlinear coupling strength can be adjusted conveniently by changing the coherent drive field. As an example, we apply this model to predict and describe phonon blockade in a nanomechanical resonator coupled to a Cooper-pair box (i.e., a charge qubit) with a linear longitudinal coupling. By obtaining the solutions of the steady state for this composite system, we give the conditions for observing strong antibunching and sub-Poissonian phonon-number statistics in this induced second-order nonlinear system. Besides using the qubit to produce phonon blockade states, the qubit itself can also be employed to detect blockade effects by measuring its states. Numerical simulations indicate that the robustness of the phonon blockade, and the sensitivity of detecting it, will benefit from this strong induced nonlinear coupling.

  11. Experimental observation of locally-resonant and Bragg band gaps for surface guided waves in a phononic crystal of pillars

    NASA Astrophysics Data System (ADS)

    Achaoui, Younes; Khelif, Abdelkrim; Benchabane, Sarah; Robert, Laurent; Laude, Vincent

    2011-03-01

    We report on the experimental study of the propagation of surface guided waves in a periodic arrangement of pillars on a semi-infinite medium. Samples composed of nickel pillars grown on a lithium niobate substrate were prepared and wide bandwidth transducers were used for the electrical generation of surface elastic waves. We identify a complete band gap for surface guided waves appearing at frequencies markedly lower than the Bragg band gap. Using optical measurements of the surface vibrations and by comparison with a finite element model, we argue that the low frequency band gap arises because of local resonances in the pillars. When resonance is reached, the acoustic energy is confined inside the pillars and transmission through the array is strongly reduced. At higher frequencies and inside the Bragg band gap, the incident surface elastic waves are almost completely reflected and the observed exponential decay of the transmission is similar to the case of phononic crystals made of holes in a substrate.

  12. Study of the optical phonons on gated twisted bilayer graphene

    NASA Astrophysics Data System (ADS)

    Chung, Ting Fung; He, Rui; Wu, Tai-Lung; Chen, Yong P.

    2015-03-01

    In twisted bilayer graphene (tBLG), the low-energy van-Hove singularities (vHs) in the density of states (DOS) can be continuously tuned by twisting the two layers, leading to distinct electronic and optical properties compared to Bernal-stacked BLG (AB-BLG). This effect has been explored using resonance Raman scattering, showing enhanced Raman G and ZO' (low frequency, layer breathing vibration) bands when the vHs energy resonates with excitation laser energy. We have studied the influence on vHs and Raman bands in gated tBLG devices (at resonant twist angle ~13° under a 532 nm laser light). We observed that the G band splits with increasing doping, attributed to asymmetric doping of charge carriers in the two layers. The strongly quenched G band intensity at high doping level is ascribed to the suppression of resonant interband transitions between the two saddle points (in conduction and valence bands) which are displaced in the momentum space by gate-tuning. We have also measured the doping dependence of ZO' band and R band in tBLG. Our results demonstrate that electric-field can be used to tune the optoelectronic and vibrational properties in tBLG devices.

  13. Elastic scattering by hot electrons and apparent lifetime of longitudinal optical phonons in gallium nitride

    SciTech Connect

    Khurgin, Jacob B.; Bajaj, Sanyam; Rajan, Siddharth

    2015-12-28

    Longitudinal optical (LO) phonons in GaN generated in the channel of high electron mobility transistors (HEMT) are shown to undergo nearly elastic scattering via collisions with hot electrons. The net result of these collisions is the diffusion of LO phonons in the Brillouin zone causing reduction of phonon and electron temperatures. This previously unexplored diffusion mechanism explicates how an increase in electron density causes reduction of the apparent lifetime of LO phonons, obtained from the time resolved Raman studies and microwave noise measurements, while the actual decay rate of the LO phonons remains unaffected by the carrier density. Therefore, the saturation velocity in GaN HEMT steadily declines with increased carrier density, in a qualitative agreement with experimental results.

  14. Topological phononic states of underwater sound based on coupled ring resonators

    NASA Astrophysics Data System (ADS)

    He, Cheng; Li, Zheng; Ni, Xu; Sun, Xiao-Chen; Yu, Si-Yuan; Lu, Ming-Hui; Liu, Xiao-Ping; Chen, Yan-Feng

    2016-01-01

    We report a design of topological phononic states for underwater sound using arrays of acoustic coupled ring resonators. In each individual ring resonator, two degenerate acoustic modes, corresponding to clockwise and counter-clockwise propagation, are treated as opposite pseudospins. The gapless edge states arise in the bandgap resulting in protected pseudospin-dependent sound transportation, which is a phononic analogue of the quantum spin Hall effect. We also investigate the robustness of the topological sound state, suggesting that the observed pseudospin-dependent sound transportation remains unless the introduced defects facilitate coupling between the clockwise and counter-clockwise modes (in other words, the original mode degeneracy is broken). The topological engineering of sound transportation will certainly promise unique design for next generation of acoustic devices in sound guiding and switching, especially for underwater acoustic devices.

  15. Analytic band Monte Carlo model for electron transport in Si including acoustic and optical phonon dispersion

    NASA Astrophysics Data System (ADS)

    Pop, Eric; Dutton, Robert W.; Goodson, Kenneth E.

    2004-11-01

    We describe the implementation of a Monte Carlo model for electron transport in silicon. The model uses analytic, nonparabolic electron energy bands, which are computationally efficient and sufficiently accurate for future low-voltage (<1V) nanoscale device applications. The electron-lattice scattering is incorporated using an isotropic, analytic phonon-dispersion model, which distinguishes between the optical/acoustic and the longitudinal/transverse phonon branches. We show that this approach avoids introducing unphysical thresholds in the electron distribution function, and that it has further applications in computing detailed phonon generation spectra from Joule heating. A set of deformation potentials for electron-phonon scattering is introduced and shown to yield accurate transport simulations in bulk silicon across a wide range of electric fields and temperatures. The shear deformation potential is empirically determined at Ξu=6.8eV, and consequently, the isotropically averaged scattering potentials with longitudinal and transverse acoustic phonons are DLA=6.39eV and DTA=3.01eV, respectively, in reasonable agreement with previous studies. The room-temperature electron mobility in strained silicon is also computed and shown to be in better agreement with the most recent phonon-limited data available. As a result, we find that electron coupling with g-type phonons is about 40% lower, and the coupling with f-type phonons is almost twice as strong as previously reported.

  16. Resonant electron heating and molecular phonon cooling in single C60 junctions.

    PubMed

    Schulze, G; Franke, K J; Gagliardi, A; Romano, G; Lin, C S; Rosa, A L; Niehaus, T A; Frauenheim, Th; Di Carlo, A; Pecchia, A; Pascual, J I

    2008-04-01

    We study heating and heat dissipation of a single C(60) molecule in the junction of a scanning tunneling microscope by measuring the electron current required to thermally decompose the fullerene cage. The power for decomposition varies with electron energy and reflects the molecular resonance structure. When the scanning tunneling microscope tip contacts the fullerene the molecule can sustain much larger currents. Transport simulations explain these effects by molecular heating due to resonant electron-phonon coupling and molecular cooling by vibrational decay into the tip upon contact formation. PMID:18517981

  17. Optically detected magnetic resonance imaging

    SciTech Connect

    Blank, Aharon; Shapiro, Guy; Fischer, Ran; London, Paz; Gershoni, David

    2015-01-19

    Optically detected magnetic resonance provides ultrasensitive means to detect and image a small number of electron and nuclear spins, down to the single spin level with nanoscale resolution. Despite the significant recent progress in this field, it has never been combined with the power of pulsed magnetic resonance imaging techniques. Here, we demonstrate how these two methodologies can be integrated using short pulsed magnetic field gradients to spatially encode the sample. This result in what we denote as an 'optically detected magnetic resonance imaging' technique. It offers the advantage that the image is acquired in parallel from all parts of the sample, with well-defined three-dimensional point-spread function, and without any loss of spectroscopic information. In addition, this approach may be used in the future for parallel but yet spatially selective efficient addressing and manipulation of the spins in the sample. Such capabilities are of fundamental importance in the field of quantum spin-based devices and sensors.

  18. Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter

    SciTech Connect

    Ceban, V. Macovei, M. A.

    2015-11-15

    The concept of an acoustical analog of the optical laser has been developed recently in both theoretical and experimental works. We here discuss a model of a coherent phonon generator with a direct signature of the quantum properties of sound vibrations. The considered setup is made of a laser-driven quantum dot embedded in an acoustical nanocavity. The system dynamics is solved for a single phonon mode in the steady-state and in the strong quantum dot—phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e., is sub-Poissonian.

  19. Spectrally resolved detection in transient-reflectivity measurements of coherent optical phonons in diamond

    NASA Astrophysics Data System (ADS)

    Nakamura, Kazutaka G.; Ohya, Kazuma; Takahashi, Hiroshi; Tsuruta, Tetsuya; Sasaki, Hiroya; Uozumi, Shin-ichi; Norimatsu, Katsura; Kitajima, Masahiro; Shikano, Yutaka; Kayanuma, Yosuke

    2016-07-01

    Coherent optical phonons in bulk solid systems play a crucial role in understanding and designing light-matter interactions and can be detected by the transient-reflectivity measurement. In this paper, we demonstrate spectrally resolved detection of coherent optical phonons in diamond from ultrashort infrared pump-probe measurements using optical bandpass filters. We show that this enhances the sensitivity approximately 35 times in measuring the coherent oscillations in the transient reflectivity compared with the commonly used spectrally integrated measurement. To explain this observation, we discuss its mechanism.

  20. Effects of ternary mixed crystal and size on optical phonons in wurtzite nitride core-shell nanowires

    SciTech Connect

    Li, J.; Guan, J. Y.; Zhang, S. F.; Ban, S. L.; Qu, Y.

    2014-04-21

    Within the framework of dielectric continuum and Loudon's uniaxial crystal models, existence conditions dependent on components and frequencies for optical phonons in wurtzite nitride core-shell nanowires (CSNWs) are discussed to obtain dispersion relations and electrostatic potentials of optical phonons in In{sub x}Ga{sub 1−x}N/GaN CSNWs. The results show that there may be four types of optical phonons in In{sub x}Ga{sub 1−x}N/GaN CSNWs for a given ternary mixed crystal (TMC) component due to the phonon dispersion anisotropy. This property is analogous to wurtzite planar heterojunctions. Among the optical phonons, there are two types of quasi-confined optical (QCO) phonons (named, respectively, as QCO-A and QCO-B), one type of interface (IF) phonons and propagating (PR) phonons existing in certain component and frequency domains while the dispersion relations and electrostatic potentials of same type of optical phonons vary with components. Furthermore, the size effect on optical phonons in CSNWs is also discussed. The dispersion relations of IF and QCO-A are independent of the boundary location of CSNWs. Meanwhile, dispersion relations and electrostatic potentials of QCO-B and PR phonons vary obviously with size, especially, when the ratio of a core radius to a shell radius is small, and dispersion relation curves of PR phonons appear to be close to each other, whereas, this phenomenon disappears when the ratio becomes large. Based on our conclusions, one can further discuss photoelectric properties in nitride CSNWs consisting of TMCs associated with optical phonons.

  1. Emergence of an Out-of-Plane Optical Phonon (ZO) Kohn Anomaly in Quasifreestanding Epitaxial Graphene.

    PubMed

    Politano, Antonio; de Juan, Fernando; Chiarello, Gennaro; Fertig, Herbert A

    2015-08-14

    In neutral graphene, two prominent cusps known as Kohn anomalies are found in the phonon dispersion of the highest optical phonon at q=Γ (LO branch) and q=K (TO branch), reflecting a significant electron-phonon coupling (EPC) to undoped Dirac electrons. In this work, high-resolution electron energy loss spectroscopy is used to measure the phonon dispersion around the Γ point in quasifreestanding graphene epitaxially grown on Pt(111). The Kohn anomaly for the LO phonon is observed at finite momentum q~2k_{F} from Γ, with a shape in excellent agreement with the theory and consistent with known values of the EPC and the Fermi level. More strikingly, we also observe a Kohn anomaly at the same momentum for the out-of-plane optical phonon (ZO) branch. This observation is the first direct evidence of the coupling of the ZO mode with Dirac electrons, which is forbidden for freestanding graphene but becomes allowed in the presence of a substrate. Moreover, we estimate the EPC to be even greater than that of the LO mode, making graphene on Pt(111) an optimal system to explore the effects of this new coupling in the electronic properties. PMID:26317732

  2. Optical-phonon-mediated photocurrent in terahertz quantum-well photodetectors

    SciTech Connect

    Gu, L. L.; Guo, X. G. Fu, Z. L.; Wan, W. J.; Zhang, R.; Tan, Z. Y.; Cao, J. C.

    2015-03-16

    Strong and sharp photocurrent peak at longitudinal optical (LO) phonon frequency (8.87 THz) is found in GaAs/(Al,Ga)As terahertz quantum-well photodetectors (QWPs). Two mesa-structure terahertz QWPs with and without one-dimensional metal grating are fabricated to investigate the behavior of such photoresponse peak. The experimental and simulation results indicate that the photocurrent peak originates from a two-step process. First, at the LO phonon frequency, a large number of non-equilibrium LO phonons are excited by the incident electromagnetic field, and the electromagnetic energy is localized and enhanced in the thin multi-quantum-well layer. Second, through the Frohlich interaction, the localized electrons are excited to continuum states by absorbing the non-equilibrium LO phonons, which leads to the strong photoresponse peak. This finding is useful for exploring strong light-matter interaction and realizing high sensitive terahertz photodetectors.

  3. Instability of insulating states in optical lattices due to collective phonon excitations

    NASA Astrophysics Data System (ADS)

    Yukalov, V. I.; Ziegler, K.

    2015-02-01

    The effect of collective phonon excitations on the properties of cold atoms in optical lattices is investigated. These phonon excitations are collective excitations, whose appearance is caused by intersite atomic interactions correlating the atoms, and they do not arise without such interactions. These collective excitations should not be confused with lattice vibrations produced by an external force. No such force is assumed. But the considered phonons are purely self-organized collective excitations, characterizing atomic oscillations around lattice sites, due to intersite atomic interactions. It is shown that these excitations can essentially influence the possibility of atoms' being localized. The states that would be insulating in the absence of phonon excitations can become delocalized when these excitations are taken into account. This concerns long-range as well as local atomic interactions. To characterize the region of stability, the Lindemann criterion is used.

  4. Interaction of optical and interface phonons and their anisotropy in GaAs/AlAs superlattices: Experiment and calculations

    SciTech Connect

    Volodin, V. A.; Sachkov, V. A.; Sinyukov, M. P.

    2015-05-15

    The angular anisotropy of interface phonons and their interaction with optical phonons in (001) GaAs/AlAs superlattices are calculated and experimentally studied. Experiments were performed by Raman light scattering in different scattering geometries for phonons with the wave vector directed normally to the superlattice and along its layers. Phonon frequencies were calculated by the extended Born method taking the Coulomb interaction into account in the rigid-ion approximation. Raman scattering spectra were calculated in the Volkenshtein bond-polarizability approximation. Calculations confirmed that the angular anisotropy of phonons observed in experiments appears due to interaction (mixing) of optical phonons, in which atoms are mainly displaced normally to superlattices, with interface phonons (TO-IF modes). In the scattering geometry, when the wave vector lies in the plane of superlattice layers, the mixed TO-IF modes are observed under nonresonance conditions. The Raman spectra for TO-IF modes depend on the mixing of atoms at heteroboundaries.

  5. Blocking Phonon Transport by Structural Resonances in Alloy-Based Nanophononic Metamaterials Leads to Ultralow Thermal Conductivity

    NASA Astrophysics Data System (ADS)

    Xiong, Shiyun; Sääskilahti, Kimmo; Kosevich, Yuriy A.; Han, Haoxue; Donadio, Davide; Volz, Sebastian

    2016-07-01

    Understanding the design rules to obtain materials that enable a tight control of phonon transport over a broad range of frequencies would aid major developments in thermoelectric energy harvesting, heat management in microelectronics, and information and communication technology. Using atomistic simulations we show that the metamaterials approach relying on localized resonances is very promising to engineer heat transport at the nanoscale. Combining designed resonant structures to alloying can lead to extremely low thermal conductivity in silicon nanowires. The hybridization between resonant phonons and propagating modes greatly reduces the group velocities and the phonon mean free paths in the low frequency acoustic range below 4 THz. Concurrently, alloy scattering hinders the propagation of high frequency thermal phonons. Our calculations establish a rationale between the size, shape, and period of the resonant structures, and the thermal conductivity of the nanowire, and demonstrate that this approach is even effective to block phonon transport in wavelengths much longer than the size and period of the surface resonant structures. A further consequence of using resonant structures is that they are not expected to scatter electrons, which is beneficial for thermoelectric applications.

  6. Blocking Phonon Transport by Structural Resonances in Alloy-Based Nanophononic Metamaterials Leads to Ultralow Thermal Conductivity.

    PubMed

    Xiong, Shiyun; Sääskilahti, Kimmo; Kosevich, Yuriy A; Han, Haoxue; Donadio, Davide; Volz, Sebastian

    2016-07-01

    Understanding the design rules to obtain materials that enable a tight control of phonon transport over a broad range of frequencies would aid major developments in thermoelectric energy harvesting, heat management in microelectronics, and information and communication technology. Using atomistic simulations we show that the metamaterials approach relying on localized resonances is very promising to engineer heat transport at the nanoscale. Combining designed resonant structures to alloying can lead to extremely low thermal conductivity in silicon nanowires. The hybridization between resonant phonons and propagating modes greatly reduces the group velocities and the phonon mean free paths in the low frequency acoustic range below 4 THz. Concurrently, alloy scattering hinders the propagation of high frequency thermal phonons. Our calculations establish a rationale between the size, shape, and period of the resonant structures, and the thermal conductivity of the nanowire, and demonstrate that this approach is even effective to block phonon transport in wavelengths much longer than the size and period of the surface resonant structures. A further consequence of using resonant structures is that they are not expected to scatter electrons, which is beneficial for thermoelectric applications. PMID:27447516

  7. Wavelength-tunable optical ring resonators

    DOEpatents

    Watts, Michael R.; Trotter, Douglas C.; Young, Ralph W.; Nielson, Gregory N.

    2009-11-10

    Optical ring resonator devices are disclosed that can be used for optical filtering, modulation or switching, or for use as photodetectors or sensors. These devices can be formed as microdisk ring resonators, or as open-ring resonators with an optical waveguide having a width that varies adiabatically. Electrical and mechanical connections to the open-ring resonators are made near a maximum width of the optical waveguide to minimize losses and thereby provide a high resonator Q. The ring resonators can be tuned using an integral electrical heater, or an integral semiconductor junction.

  8. Wavelength-tunable optical ring resonators

    DOEpatents

    Watts, Michael R.; Trotter, Douglas C.; Young, Ralph W.; Nielson, Gregory N.

    2011-07-19

    Optical ring resonator devices are disclosed that can be used for optical filtering, modulation or switching, or for use as photodetectors or sensors. These devices can be formed as microdisk ring resonators, or as open-ring resonators with an optical waveguide having a width that varies adiabatically. Electrical and mechanical connections to the open-ring resonators are made near a maximum width of the optical waveguide to minimize losses and thereby provide a high resonator Q. The ring resonators can be tuned using an integral electrical heater, or an integral semiconductor junction.

  9. Coherent phonon spectroscopy of non-fully symmetric modes using resonant terahertz excitation

    SciTech Connect

    Huber, T. Huber, L.; Johnson, S. L.; Ranke, M.; Ferrer, A.

    2015-08-31

    We use intense terahertz (THz) frequency electromagnetic pulses generated via optical rectification in an organic crystal to drive vibrational lattice modes in single crystal Tellurium. The coherent modes are detected by measuring the polarization changes of femtosecond laser pulses reflecting from the sample surface, resulting in a phase-resolved detection of the coherent lattice motion. We compare the data to a model of Lorentz oscillators driven by the near-single-cycle broadband THz pulse. The demonstrated technique of optically probed coherent phonon spectroscopy with THz frequency excitation could prove to be a viable alternative to other time-resolved spectroscopic methods like standard THz time domain spectroscopy.

  10. Coherent phonon spectroscopy of non-fully symmetric modes using resonant terahertz excitation

    NASA Astrophysics Data System (ADS)

    Huber, T.; Ranke, M.; Ferrer, A.; Huber, L.; Johnson, S. L.

    2015-08-01

    We use intense terahertz (THz) frequency electromagnetic pulses generated via optical rectification in an organic crystal to drive vibrational lattice modes in single crystal Tellurium. The coherent modes are detected by measuring the polarization changes of femtosecond laser pulses reflecting from the sample surface, resulting in a phase-resolved detection of the coherent lattice motion. We compare the data to a model of Lorentz oscillators driven by the near-single-cycle broadband THz pulse. The demonstrated technique of optically probed coherent phonon spectroscopy with THz frequency excitation could prove to be a viable alternative to other time-resolved spectroscopic methods like standard THz time domain spectroscopy.

  11. Optical coherence in atomic monolayer transition metal dichalcogenides limited by electron-phonon interactions

    NASA Astrophysics Data System (ADS)

    Dey, Prasenjit; Paul, Jagannath; Wang, Zefang; Stevens, Christopher; Liu, Cunming; Romero, Aldo; Shan, Jie; Hilton, David; Karaiskaj, Denis; Aldo Romero Collaboration; Zefang Wang, Jie Shan Collaboration; David HIlton Collaboration

    We systematically investigate the excitonic dephasing of three representative transition metal dichalcogenides, namely MoS2, MoSe2 and WSe2 atomic monolayer thick and bulk crystals, in order to gain proper understanding of the factors that determine the optical coherence in these materials. Coherent nonlinear optical spectroscopy, temperature dependent absorption combined with `ab initio' theoretical calculations of the phonon spectra, indicate electron-phonon interactions to be the limiting factor. The research at USF, Penn. State, and UAB is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-SC0012635.

  12. Imaging carrier and phonon transport in Si using ultrashort optical pulses

    SciTech Connect

    David H. Hurley; O. B. Wright; O. Matsuda; B. E. McCandless; S. Shinde

    2009-01-01

    A series of experiments have been conducted that microscopically image thermal diffusion and surface acoustic phonon propagation within a single crystallite of a polycrystalline Si sample. The experimental approach employs ultrashort optical pulses to generate an electron-hole plasma and a second probe pulse is used to image the evolution of the plasma. By decomposing the signal into a component that varies with delay time and a steady state component that varies with pump modulation frequency, the respective influence of carrier recombination and thermal diffusion are identified. Additionally, the coherent surface acoustic phonon component to the signal is imaged using a Sagnac interferometer to monitor optical phase.

  13. Multilayer-split-tube resonators with low-frequency band gaps in phononic crystals

    NASA Astrophysics Data System (ADS)

    Jing, Li; Wu, Jiu Hui; Guan, Dong; Gao, Nansha

    2014-09-01

    In this paper, low-frequency band gaps in two-dimensional Helmholtz resonant phononic crystals (PCs) composed of multilayer-split-tube resonators are investigated. The band structures, transmission spectra, and pressure field of the acoustic modes of these PCs are calculated by using a finite element method (FEM). The numerical results show that the first band gap of the structure is from 88 to 140 Hz. The transmission spectra are in accordance with those of the dispersion relation calculations. The acoustic modes of the bands are analyzed to reveal the nature of this phenomenon. It is found that the interaction between the local resonance and the traveling wave modes in proposed structure is responsible for the formation of the first band gap. The influences of the structural parameters on the band gaps are investigated by using FEM and the electrical circuit analogy. Numerical results show that the band gaps can be modulated in an even wider frequency range by changing the structural parameters, such as the rotation angle, the number of tubes, and the radius of the outer tube. The structural design results provide an effective way for phononic crystals to obtain the low-frequency band gaps, which have potential application in the low-frequency noise reduction.

  14. Isoscalar and isovector giant resonances in a self-consistent phonon coupling approach

    NASA Astrophysics Data System (ADS)

    Lyutorovich, N.; Tselyaev, V.; Speth, J.; Krewald, S.; Grümmer, F.; Reinhard, P.-G.

    2015-10-01

    We present fully self-consistent calculations of isoscalar giant monopole and quadrupole as well as isovector giant dipole resonances in heavy and light nuclei. The description is based on Skyrme energy-density functionals determining the static Hartree-Fock ground state and the excitation spectra within random-phase approximation (RPA) and RPA extended by including the quasiparticle-phonon coupling at the level of the time-blocking approximation (TBA). All matrix elements were derived consistently from the given energy-density functional and calculated without any approximation. As a new feature in these calculations, the single-particle continuum was included thus avoiding the artificial discretization usually implied in RPA and TBA. The step to include phonon coupling in TBA leads to small, but systematic, down shifts of the centroid energies of the giant resonances. These shifts are similar in size for all Skyrme parametrizations investigated here. After all, we demonstrate that one can find Skyrme parametrizations which deliver a good simultaneous reproduction of all three giant resonances within TBA.

  15. Hyperbolic phonon-polaritons in boron nitride for near-field optical imaging and focusing

    NASA Astrophysics Data System (ADS)

    Li, Peining; Lewin, Martin; Kretinin, Andrey V.; Caldwell, Joshua D.; Novoselov, Kostya S.; Taniguchi, Takashi; Watanabe, Kenji; Gaussmann, Fabian; Taubner, Thomas

    2015-06-01

    Hyperbolic materials exhibit sub-diffractional, highly directional, volume-confined polariton modes. Here we report that hyperbolic phonon polaritons allow for a flat slab of hexagonal boron nitride to enable exciting near-field optical applications, including unusual imaging phenomenon (such as an enlarged reconstruction of investigated objects) and sub-diffractional focusing. Both the enlarged imaging and the super-resolution focusing are explained based on the volume-confined, wavelength dependent propagation angle of hyperbolic phonon polaritons. With advanced infrared nanoimaging techniques and state-of-art mid-infrared laser sources, we have succeeded in demonstrating and visualizing these unexpected phenomena in both Type I and Type II hyperbolic conditions, with both occurring naturally within hexagonal boron nitride. These efforts have provided a full and intuitive physical picture for the understanding of the role of hyperbolic phonon polaritons in near-field optical imaging, guiding, and focusing applications.

  16. Hyperbolic phonon-polaritons in boron nitride for near-field optical imaging and focusing.

    PubMed

    Li, Peining; Lewin, Martin; Kretinin, Andrey V; Caldwell, Joshua D; Novoselov, Kostya S; Taniguchi, Takashi; Watanabe, Kenji; Gaussmann, Fabian; Taubner, Thomas

    2015-01-01

    Hyperbolic materials exhibit sub-diffractional, highly directional, volume-confined polariton modes. Here we report that hyperbolic phonon polaritons allow for a flat slab of hexagonal boron nitride to enable exciting near-field optical applications, including unusual imaging phenomenon (such as an enlarged reconstruction of investigated objects) and sub-diffractional focusing. Both the enlarged imaging and the super-resolution focusing are explained based on the volume-confined, wavelength dependent propagation angle of hyperbolic phonon polaritons. With advanced infrared nanoimaging techniques and state-of-art mid-infrared laser sources, we have succeeded in demonstrating and visualizing these unexpected phenomena in both Type I and Type II hyperbolic conditions, with both occurring naturally within hexagonal boron nitride. These efforts have provided a full and intuitive physical picture for the understanding of the role of hyperbolic phonon polaritons in near-field optical imaging, guiding, and focusing applications. PMID:26112474

  17. Hyperbolic phonon-polaritons in boron nitride for near-field optical imaging and focusing

    PubMed Central

    Li, Peining; Lewin, Martin; Kretinin, Andrey V.; Caldwell, Joshua D.; Novoselov, Kostya S.; Taniguchi, Takashi; Watanabe, Kenji; Gaussmann, Fabian; Taubner, Thomas

    2015-01-01

    Hyperbolic materials exhibit sub-diffractional, highly directional, volume-confined polariton modes. Here we report that hyperbolic phonon polaritons allow for a flat slab of hexagonal boron nitride to enable exciting near-field optical applications, including unusual imaging phenomenon (such as an enlarged reconstruction of investigated objects) and sub-diffractional focusing. Both the enlarged imaging and the super-resolution focusing are explained based on the volume-confined, wavelength dependent propagation angle of hyperbolic phonon polaritons. With advanced infrared nanoimaging techniques and state-of-art mid-infrared laser sources, we have succeeded in demonstrating and visualizing these unexpected phenomena in both Type I and Type II hyperbolic conditions, with both occurring naturally within hexagonal boron nitride. These efforts have provided a full and intuitive physical picture for the understanding of the role of hyperbolic phonon polaritons in near-field optical imaging, guiding, and focusing applications. PMID:26112474

  18. Reversible optical switching of highly confined phonon-polaritons with an ultrathin phase-change material.

    PubMed

    Li, Peining; Yang, Xiaosheng; Maß, Tobias W W; Hanss, Julian; Lewin, Martin; Michel, Ann-Katrin U; Wuttig, Matthias; Taubner, Thomas

    2016-08-01

    Surface phonon-polaritons (SPhPs), collective excitations of photons coupled with phonons in polar crystals, enable strong light-matter interaction and numerous infrared nanophotonic applications. However, as the lattice vibrations are determined by the crystal structure, the dynamical control of SPhPs remains challenging. Here, we realize the all-optical, non-volatile, and reversible switching of SPhPs by controlling the structural phase of a phase-change material (PCM) employed as a switchable dielectric environment. We experimentally demonstrate optical switching of an ultrathin PCM film (down to 7 nm, <λ/1,200) with single laser pulses and detect ultra-confined SPhPs (polariton wavevector kp > 70k0, k0 = 2π/λ) in quartz. Our proof of concept allows the preparation of all-dielectric, rewritable SPhP resonators without the need for complex fabrication methods. With optimized materials and parallelized optical addressing we foresee application potential for switchable infrared nanophotonic elements, for example, imaging elements such as superlenses and hyperlenses, as well as reconfigurable metasurfaces and sensors. PMID:27213955

  19. Optical phonon modes in rhombohedral boron monosulfide under high pressure

    SciTech Connect

    Cherednichenko, Kirill A.; Sokolov, Petr S.; Solozhenko, Vladimir L.; Kalinko, Aleksandr; Le Godec, Yann; Polian, Alain; Itié, Jean-Paul

    2015-05-14

    Raman spectra of rhombohedral boron monosulfide (r-BS) were measured under pressures up to 34 GPa at room temperature. No pressure-induced structural phase transition was observed, while strong pressure shift of Raman bands towards higher wavenumbers has been revealed. IR spectroscopy as a complementary technique has been used in order to completely describe the phonon modes of r-BS. All experimentally observed bands have been compared with theoretically calculated ones and modes assignment has been performed. r-BS enriched by {sup 10}B isotope was synthesized, and the effect of boron isotopic substitution on Raman spectra was observed and analyzed.

  20. Optical Phonons In InAlAs Thin Layers: Raman And IR Study

    SciTech Connect

    Milekhin, A.; Kalagin, A.; Vasilenko, A.; Toropov, A.; Surovtsev, N.; Zahn, D. R. T.

    2010-01-04

    We present a study of the optical phonon spectrum of relaxed In{sub x}Al{sub 1-x}As epitaxial layers grown by molecular-beam epitaxy on GaAs substrates in the whole range of In content (x = 0 divide 1) using macro- and micro-Raman and IR spectroscopies.

  1. Mechanism of current modulation by optic phonon emission in heterojunction tunneling experiments

    SciTech Connect

    Hanna, C.B.; Hellman, E.S.; Laughlin, R.B.

    1985-08-27

    We explain recent observations by Hickmott et al. of sequential longitudinal optic phonon emission in tunneling currents of GaAs-Al/sub x/Ga/sub 1-x/As heterojunctions in terms of inhomogeneous tunneling and a magnetopolaronic mass correction. 16 refs., 13 figs.

  2. Phonon-mediated squeezing of the cavity field off-resonantly coupled with a coherently driven quantum dot

    SciTech Connect

    Zhu, Jia-pei; Huang, Hui; Li, Gao-xiang

    2014-01-21

    We theoretically propose a scheme for the quadrature squeezing of the cavity field via dissipative processes. The effects of the electron-phonon interaction (EPI) on the squeezing are investigated, where the cavity is off-resonantly coupled with a coherently driven quantum dot (QD) which is allowed to interact with an acoustic-phonon reservoir. Under certain conditions, the participation of the phonon induced by both the EPI and the off-resonant coupling of the cavity with the QD enables some dissipative processes to occur resonantly in the dressed-state basis of the QD. The cavity-mode photons emitted or absorbed during the phonon-mediated dissipative processes are correlated, thus leading to the squeezing of the cavity field. A squeezed vacuum reservoir for the cavity field is built up due to the EPI plus the off-resonant coupling between the cavity and the QD. The numerical results obtained with an effective polaron master equation derived using second-order perturbation theory indicate that, in low temperature limit, the degree of squeezing is maximal but the increasing temperature of the phonon reservoir could hinder the squeezing and degrade the degree of the squeezing of the cavity field. In addition, the presence of the photonic crystal could enhance the quadrature squeezing of the cavity field.

  3. Excitons in one-phonon resonant Raman scattering: Fröhlich and interference effects

    NASA Astrophysics Data System (ADS)

    Cantarero, A.; Trallero-Giner, C.; Cardona, M.

    1989-12-01

    A theoretical model of resonant Raman scattering including excitons as intermediate states in the process is compared with recent experimental results in some III-V compound semiconductors where the Raman polarizability was obtained in absolute value for several scattering configurations. In particular, Fröhlich (F) interaction and its interference with the deformation potential (DP) one is analyzed in the E0+Δ0 critical point (CP) of GaAs at three different temperatures. Also the E0 and E0+Δ0 CP of GaP and E0+Δ0 of GaSb are analyzed. We show that the inclusion of impurity-induced forbidden LO-phonon Raman scattering is not necessary when excitonic effects are considered. The experimental data of GaAs corresponding to F interaction can be fitted by assuming a Fröhlich constant cF=0.14 eV Aṥ/2. Lifetime broadenings of 12 meV (10 K), 14 meV (100 K), and 28 meV (300 K) are deduced. The lifetime broadening of GaAs and GaSb at 100 K are taken from two-phonon Raman scattering spectra where the incoming and outgoing resonances are well defined. The general features in the comparison with the experiment is that the measured spectra corresponding to F interaction are well fitted; however, the theoretical interference is stronger than the measured one.

  4. Optical and Phonon Characterization of Ternary CdSe x S1- x Alloy Quantum Dots

    NASA Astrophysics Data System (ADS)

    Thi, L. A.; Cong, N. D.; Dang, N. T.; Nghia, N. X.; Quang, V. X.

    2016-05-01

    Ternary CdSe x S1- x alloy quantum dots (QDs) were synthesized using a wet chemical method. Their morphology, particle size, structural, optical, and vibrational properties were investigated using transmission electron microscopy, x-ray diffraction, UV-Vis, fluorescence and Raman spectroscopy, respectively. The optical and vibrational properties of the QDs can be controlled by adjusting the Se/S molar ratio. The absorption and emission peaks shift to a longer wavelength range when increasing the Se content. The presence of two CdSe-like and CdS-like longitudinal optical phonon modes was observed. The dependencies of the optical and phonon modes on the Se content are discussed in detail.

  5. High-speed asynchronous optical sampling for high-sensitivity detection of coherent phonons

    NASA Astrophysics Data System (ADS)

    Dekorsy, T.; Taubert, R.; Hudert, F.; Schrenk, G.; Bartels, A.; Cerna, R.; Kotaidis, V.; Plech, A.; Köhler, K.; Schmitz, J.; Wagner, J.

    2007-12-01

    A new optical pump-probe technique is implemented for the investigation of coherent acoustic phonon dynamics in the GHz to THz frequency range which is based on two asynchronously linked femtosecond lasers. Asynchronous optical sampling (ASOPS) provides the performance of on all-optical oscilloscope and allows us to record optically induced lattice dynamics over nanosecond times with femtosecond resolution at scan rates of 10 kHz without any moving part in the set-up. Within 1 minute of data acquisition time signal-to-noise ratios better than 107 are achieved. We present examples of the high-sensitivity detection of coherent phonons in superlattices and of the coherent acoustic vibration of metallic nanoparticles.

  6. Optical Microspherical Resonators for Biomedical Sensing

    PubMed Central

    Soria, Silvia; Berneschi, Simone; Brenci, Massimo; Cosi, Franco; Conti, Gualtiero Nunzi; Pelli, Stefano; Righini, Giancarlo C.

    2011-01-01

    Optical resonators play an ubiquitous role in modern optics. A particular class of optical resonators is constituted by spherical dielectric structures, where optical rays are total internal reflected. Due to minimal reflection losses and to potentially very low material absorption, these guided modes, known as whispering gallery modes, can confer the resonator an exceptionally high quality factor Q, leading to high energy density, narrow resonant-wavelength lines and a lengthy cavity ringdown. These attractive characteristics make these miniaturized optical resonators especially suited as laser cavities and resonant filters, but also as very sensitive sensors. First, a brief analysis is presented of the characteristics of microspherical resonators, of their fabrication methods, and of the light coupling techniques. Then, we attempt to overview some of the recent advances in the development of microspherical biosensors, underlining a number of important applications in the biomedical field. PMID:22346603

  7. Waveguide-coupled surface phonon resonance sensors with super-resolution in the mid-infrared region.

    PubMed

    Zheng, Gaige; Chen, Yunyun; Bu, Lingbing; Xu, Linhua; Su, Wei

    2016-04-01

    A waveguide-coupled surface phonon resonance (SPhR) sensor with super-resolution based on Fano resonance (FR) by using a multilayer system within the Kretschmann configuration in the mid-infrared wavelength region is proposed. Due to the coherent interference of the waveguide and the surface phonon polariton modes, the calculated reflectivity spectrum possesses sharp asymmetric FR dips. An ultra-small linewidth is formed because of the Fano coupling, and the physical features contribute to a highly efficient nano-sensor for refractive index sensing. The bulk and surface sensitivity by intensities are greatly enhanced relative to those of conventional SPhR sensors. PMID:27192292

  8. Coupled bipolarons and optical phonons as a model for high-T(sub c) superconductors

    NASA Technical Reports Server (NTRS)

    Kasperczyk, J.

    1990-01-01

    The coherence length of the new high-temperature superconductors reaches very small value which is comparable to the dimensions of unit cell of these compounds. This means that a pair consists of two holes occupying the same site or two adjacent sites. Such a situation seems to be described by a model of the local-pairs (bipolarons). The origin of local-pairs may come not only from strong enough electron or hole-phonon interaction but also from other interactions. Independent of the specific nature of such local-pairs, they can undergo a Bose-like condensation to the superconducting state at a critical temperature which is usually much lower than the temperature of the pair formation. An interplay of ferroelectric and superconducting properties is considered within the model of hole-like local-pairs interacting with optical phonons. Therefore, researchers extend the usual local-pair Hamiltonian by including a direct interaction between the local-pairs and the optical phonons. These optical phonons are known to play an important role in the ferroelectric transition, if any, and they transform into an additional pseudo-acoustic branch at the ferroelectric critical temperature. (This is associated with nonzero electric polarization due to the existence of two separate lattices composed of negative and positive ions, respectively.)

  9. Coupled bipolarons and optical phonons as a model for high-Tc superconductors

    NASA Technical Reports Server (NTRS)

    Kasperczyk, J.

    1991-01-01

    The coherence length of the new high-temperature superconductors reaches a small value which is comparable to the dimensions of the unit cell of the compound. This means that a pair consists of two holes occupying the same site or two adjacent sites. Such a situation is described by a model of the local-pairs (bipolarons). The origin of local-pairs may come not only from strong enough electron or hole-phonon interaction but also from other interactions. Independent of the specific nature of such local-pairs, they can undergo a Bose-like condensation to the superconducting state at a critical temperature which is usually much lower than the temperature of the pair formation. An interplay of ferroelectric and superconducting properties is considered within the model of hole-like local-pairs interacting with optical phonons. Therefore, researchers extend the usual local-pair Hamiltonian by including a direct interaction between the local-pairs and the optical phonons. These optical phonons are known to play an important role in the ferroelectric transition and they transform into an additional pseudo-acoustic branch at the ferroelectric critical temperature. (This is associated with nonzero electric polarization due to the existence of two separate lattices composed of negative and positive ions, respectively.)

  10. Raman Scattering from Surface Optic Phonons in Cylindrical and Rectangular Cross-sectional Semiconducting Nanowires†

    NASA Astrophysics Data System (ADS)

    Xiong, Qihua; Eklund, P. C.

    2005-03-01

    Raman scattering from surface optic (SO) phonons has been observed and identified in cylindrical GaP and rectangular cross-section ZnS nanowires. We propose that the symmetry breaking mechanism which activates the SO phonon is a periodic modulation of the cross-sectional area along the nanowires. In the case of cylindrical GaP nanowires, Raman scattering from SO phonons in air at room temperature is observed at 394 cm-1, in between the first order longitudinal optic (LO) (401 cm-1) and transverse optic (TO) (367 cm-1), and downshift to 392 cm-1 in dichloromethane (?m=2.0) and 390 cm-1 in aniline (?m=2.56). Raman scattering from the ZnS nanowires in air at room temperature reveals a strong first-order LO mode at 346 cm-1 and two TO modes at 269 and 282 cm-1. The SO Raman band in ZnS is observed at 335 cm-1 in air, and downshifts to 328 cm-1 in dichloromethane and to 326 cm-1 in aniline. The position of the SO band in GaP and ZnS nanowires is consistent with a dielectric continuum model. Theoretical SO phonon dispersion for both cylindrical and rectangular cross-section nanowires is presented and compared to experiment. This work was supported by the NSF NIRT program (DMR- 0304178).

  11. Raman study of surface optical phonons in hydrothermally obtained ZnO(Mn) nanoparticles

    NASA Astrophysics Data System (ADS)

    Hadžić, B.; Romčević, N.; Romčević, M.; Kuryliszyn-Kudelska, I.; Dobrowolski, W.; Narkiewicz, U.; Sibera, D.

    2016-08-01

    Nanocrystalline samples of ZnO(Mn) were synthesized by hydrothermal method. The morphology of the samples was studied by HRTEM and SEM. X-ray diffraction was used to determine composition of the samples (ZnO and ZnMn2O4) and the mean crystalline size (from 16 to 99 nm). In this paper we report the experimental spectra of Raman scattering (from 100 to 1600 cm-1) with surface optical phonons (SOP) in range of 497-538 cm-1 as well as formation of new phases MnO, Mn3O4 and ZnMnO3. The phonon of registered phase's exhibit effects connected to phase concentration, while the SOP phonon mode exhibit significant confinement effect.

  12. Optical phonon modes and infrared dielectric properties of monoclinic CoWO4 microcrystals

    NASA Astrophysics Data System (ADS)

    Moreira, Roberto L.; Almeida, Rafael M.; Siqueira, Kisla P. F.; Abreu, Cintia G.; Dias, Anderson

    2016-02-01

    The phonon characteristics of CoWO4 microcrystals with monoclinic Wolframite structure were investigated by far-infrared (IR) and Raman spectroscopies. Near-normal spectra were taken for IR light polarization along the principal b-axis (A u modes) and along several angles within the ac-plane (B u modes). The IR spectra were analyzed with a generalized Drude-Lorentz model, and all predicted polar phonon modes were fully determined, including their symmetries, the dielectric Lorentz parameters and the non-orthogonal phonon polarizations for the B u modes. Anomalous dispersion and negative values for the real and imaginary parts of the off-diagonal components of the dielectric tensor functions were identified and discussed under the light of the varying phonon polarization directions (spread out in the ac-plane). The obtained static and background dielectric tensors gave an average permittivity of 16.1 (at microwave region), refractive indices along the principal dielectric axes of 2.22, 2.33 and 2.44 (at 1 μm), the optical axes, and an estimated value for the biaxial angle of the crystal. Polarized Raman spectra on appropriate scattering configurations revealed the 18 non-polar gerade phonons of CoWO4 crystals, with their correct symmetries attributed.

  13. Excitons and exciton-phonon interactions in 2D MoS2 , WS2 and WSe2 studied by resonance Raman spectroscopy

    NASA Astrophysics Data System (ADS)

    Pimenta, Marcos; Del Corro, Elena; Carvalho, Bruno; Malard, Leandro; Alves, Juliana; Fantini, Cristiano; Terrones, Humberto; Elias, Ana Laura; Terrones, Mauricio

    The 2D materials exhibit a very strong exciton binding energy, and the exciton-phonon coupling plays an important role in their optical properties. Resonance Raman spectroscopy (RRS) is a very useful tool to provide information about excitons and their couplings with phonons. We will present in this work a RRS study of different samples of 2D transition metal dichalcogenides (MoS2, WS2 and WSe2) with one, two and three layers (1L, 2L, 3L) and bulk samples, using more than 30 different laser excitation lines covering the visible range. We have observed that all Raman features are enhanced by resonances with excitonic transitions. From the laser energy dependence of the Raman excitation profile (REP) we obtained the energies of the excitonic states and their dependence with the number of atomic layers.. In the case of MoS2, we observed that the electron-phonon coupling is symmetry dependent, and our results provide experimental evidence of the C exciton recently predicted theoretically. The RRS results WSe2 show that the Raman modes are enhanced by the excited excitonic states and we will present the dependence of the excited states energies on the number of layers.

  14. Resonant optical rectification in bacteriorhodopsin

    PubMed Central

    Groma, Géza I.; Colonna, Anne; Lambry, Jean-Christophe; Petrich, Jacob W.; Váró, György; Joffre, Manuel; Vos, Marten H.; Martin, Jean-Louis

    2004-01-01

    The relative role of retinal isomerization and microscopic polarization in the phototransduction process of bacteriorhodopsin is still an open question. It is known that both processes occur on an ultrafast time scale. The retinal trans→cis photoisomerization takes place on the time scale of a few hundred femtoseconds. On the other hand, it has been proposed that the primary light-induced event is a sudden polarization of the retinal environment, although there is no direct experimental evidence for femtosecond charge displacements, because photovoltaic techniques cannot be used to detect charge movements faster than picoseconds. Making use of the known high second-order susceptibility χ(2) of retinal in proteins, we have used a nonlinear technique, interferometric detection of coherent infrared emission, to study macroscopically oriented bacteriorhodopsin-containing purple membranes. We report and characterize impulsive macroscopic polarization of these films by optical rectification of an 11-fs visible light pulse in resonance with the optical transition. This finding provides direct evidence for charge separation as a precursor event for subsequent functional processes. A simple two-level model incorporating the resonant second-order optical properties of retinal, which are known to be a requirement for functioning of bacteriorhodopsin, is used to describe the observations. In addition to the electronic response, long-lived infrared emission at specific frequencies was observed, reflecting charge movements associated with vibrational motions. The simultaneous and phase-sensitive observation of both the electronic and vibrational signals opens the way to study the transduction of the initial polarization into structural dynamics. PMID:15148391

  15. Resonant optical rectification in bacteriorhodopsin.

    PubMed

    Groma, Géza I; Colonna, Anne; Lambry, Jean-Christophe; Petrich, Jacob W; Váró, György; Joffre, Manuel; Vos, Marten H; Martin, Jean-Louis

    2004-05-25

    The relative role of retinal isomerization and microscopic polarization in the phototransduction process of bacteriorhodopsin is still an open question. It is known that both processes occur on an ultrafast time scale. The retinal trans-->cis photoisomerization takes place on the time scale of a few hundred femtoseconds. On the other hand, it has been proposed that the primary light-induced event is a sudden polarization of the retinal environment, although there is no direct experimental evidence for femtosecond charge displacements, because photovoltaic techniques cannot be used to detect charge movements faster than picoseconds. Making use of the known high second-order susceptibility chi(2) of retinal in proteins, we have used a nonlinear technique, interferometric detection of coherent infrared emission, to study macroscopically oriented bacteriorhodopsin-containing purple membranes. We report and characterize impulsive macroscopic polarization of these films by optical rectification of an 11-fs visible light pulse in resonance with the optical transition. This finding provides direct evidence for charge separation as a precursor event for subsequent functional processes. A simple two-level model incorporating the resonant second-order optical properties of retinal, which are known to be a requirement for functioning of bacteriorhodopsin, is used to describe the observations. In addition to the electronic response, long-lived infrared emission at specific frequencies was observed, reflecting charge movements associated with vibrational motions. The simultaneous and phase-sensitive observation of both the electronic and vibrational signals opens the way to study the transduction of the initial polarization into structural dynamics. PMID:15148391

  16. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi, M=Ir,Os

    DOE PAGESBeta

    Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; Sales, Brian C.; Niedziela, Jennifer L.; Ma, Jie; Matsuda, Masaaki; Abernathy, Douglas L.; Berlijn, Tom

    2015-03-31

    The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe1-xMxSi (x = 0, 0.02, 0.04, 0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. In this paper, our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads tomore » softened interatomic force-constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q,E) from INS through a Green's function model incorporating the phonon self-energy based on first-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Finally, our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.« less

  17. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe 1 x M x Si (M= Ir, Os)

    DOE PAGESBeta

    Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; Sales, Brian C.; Niedziela, Jennifer L.; Ma, Jie; Matsuda, Masaaki; Abernathy, Douglas L.; Berlijn, Tom

    2015-03-31

    The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe1􀀀xMxSi (x = 0; 0:02; 0:04; 0:1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and rst-principles simulations. Our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads to softened interatomic force-constantsmore » compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q;E) from INS through a Green's function model incorporating the phonon self-energy based on rst-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.« less

  18. Onset of optical-phonon cooling in multilayer graphene revealed by RF noise and black-body radiation thermometries.

    PubMed

    Brunel, D; Berthou, S; Parret, R; Vialla, F; Morfin, P; Wilmart, Q; Fève, G; Berroir, J-M; Roussignol, P; Voisin, C; Plaçais, B

    2015-04-29

    We report on electron cooling power measurements in few-layer graphene excited by Joule heating by means of a new setup combining electrical and optical probes of the electron and phonon baths temperatures. At low bias, noise thermometry allows us to retrieve the well known acoustic phonon cooling regimes below and above the Bloch-Grüneisen temperature, with additional control over the phonon bath temperature. At high electrical bias, we show the relevance of direct optical investigation of the electronic temperature by means of black-body radiation measurements. In this regime, the onset of new efficient relaxation pathways involving optical modes is observed. PMID:25835486

  19. Opto-electronic oscillators having optical resonators

    NASA Technical Reports Server (NTRS)

    Yao, Xiaotian Steve (Inventor); Maleki, Lutfollah (Inventor); Ilchenko, Vladimir (Inventor)

    2003-01-01

    Systems and techniques of incorporating an optical resonator in an optical part of a feedback loop in opto-electronic oscillators. This optical resonator provides a sufficiently long energy storage time and hence to produce an oscillation of a narrow linewidth and low phase noise. Certain mode matching conditions are required. For example, the mode spacing of the optical resonator is equal to one mode spacing, or a multiplicity of the mode spacing, of an opto-electronic feedback loop that receives a modulated optical signal and to produce an electrical oscillating signal.

  20. Model for longitudinal-optical phonons and electron-phonon coupling in GaAs-Ga1-xAlxAs multilayer structures

    NASA Astrophysics Data System (ADS)

    Guillemot, C.; Clérot, F.

    1991-09-01

    A continuum theory is developed to investigate the properties of the long-wavelength longitudinal-optical phonons in GaAs-Ga1-xAlxAs multilayer structures and the associated electron-phonon interaction. Depending on the layer, the relative ionic displacements are related to GaAs or GaAs-type longitudinal-optical phonons and treated in the framework of the Born-Huang model, generalized to include isotropic dispersion effects in the Brillouin-zone center. For double heterostructures, a finite number of quantized confined modes is found. The interplay between the long-range Coulomb interaction, which couples the vibrations of adjacent GaAs layers, and confinement effects, which prevent the displacements of adjacent GaAs layers to overlap, is elucidated in the case of superlattices. The strength of the electron-phonon coupling in double heterostructures is reduced as compared with the electron-bulk-phonon effective coupling strength for quantum-well widths smaller than 100 Å.

  1. On-chip optical mode conversion based on dynamic grating in photonic-phononic hybrid waveguide

    PubMed Central

    Chen, Guodong; Zhang, Ruiwen; Sun, Junqiang

    2015-01-01

    We present a scheme for reversible and tunable on-chip optical mode conversion based on dynamic grating in a hybrid photonic-phononic waveguide. The dynamic grating is built up through the acousto-optic effect and the theoretical model of the optical mode conversion is developed by considering the geometrical deformation and refractive index change. Three kinds of mode conversions are able to be realized using the same hybrid waveguide structure in a large bandwidth by only changing the launched acoustic frequency. The complete mode conversion can be achieved by choosing a proper acoustic power under a given waveguide length. PMID:25996236

  2. On-chip optical mode conversion based on dynamic grating in photonic-phononic hybrid waveguide.

    PubMed

    Chen, Guodong; Zhang, Ruiwen; Sun, Junqiang

    2015-01-01

    We present a scheme for reversible and tunable on-chip optical mode conversion based on dynamic grating in a hybrid photonic-phononic waveguide. The dynamic grating is built up through the acousto-optic effect and the theoretical model of the optical mode conversion is developed by considering the geometrical deformation and refractive index change. Three kinds of mode conversions are able to be realized using the same hybrid waveguide structure in a large bandwidth by only changing the launched acoustic frequency. The complete mode conversion can be achieved by choosing a proper acoustic power under a given waveguide length. PMID:25996236

  3. Surface phonon-polariton enhanced optical forces in silicon carbide nanostructures.

    PubMed

    Li, Dongfang; Lawandy, Nabil M; Zia, Rashid

    2013-09-01

    The enhanced optical forces induced by surface phonon-polariton (SPhP) modes are investigated in different silicon carbide (SiC) nanostructures. Specifically, we calculate optical forces using the Maxwell stress tensor for three different geometries: spherical particles, slab waveguides, and rectangular waveguides. We show that SPhP modes in SiC can produce very large forces, more than one order of magnitude larger than the surface plasmon-polariton (SPP) forces in analogous metal nanostructures. The material and geometric basis for these large optical forces are examined in terms of dispersive permittivity, separation distance, and operating wavelength. PMID:24103963

  4. Magnetic resonance imaging of radiation optic neuropathy

    SciTech Connect

    Zimmerman, C.F.; Schatz, N.J.; Glaser, J.S. )

    1990-10-15

    Three patients with delayed radiation optic neuropathy after radiation therapy for parasellar neoplasms underwent magnetic resonance imaging. The affected optic nerves and chiasms showed enlargement and focal gadopentetate dimeglumine enhancement. The magnetic resonance imaging technique effectively detected and defined anterior visual pathway changes of radionecrosis and excluded the clinical possibility of visual loss because of tumor recurrence.

  5. Acoustic add-drop filters based on phononic crystal ring resonators

    NASA Astrophysics Data System (ADS)

    Rostami-Dogolsara, Babak; Moravvej-Farshi, Mohammad Kazem; Nazari, Fakhroddin

    2016-01-01

    We report the design procedure for an acoustic add-drop filter (ADF) composed of two line-defect waveguides coupled through a ring resonator cavity (RRC) all based on a phononic crystal (PnC) platform. Using finite difference time domain and plane wave expansion methods, we study the propagation of acoustic waves through the PnC based ADF structures. Numerical results show that the quality factor for the ADF with a quasisquare ring resonator with a frequency band of 95 Hz centered about 75.21 kHz is Q ˜ 800. We show that the addition of an appropriate scatterer at each RRC corner can reduce the scattering loss, enhancing the quality factor and the transmission efficiency. Moreover, it is also shown that by increasing the coupling gaps between the RRC and waveguides the quality factor can be increased by ˜25 times, at the expense of a significant reduction in the transmission efficiency this is attributed to the enhanced selectivity in expense of weakened coupling. Finally, by varying the effective path length of the acoustic wave in the RRC, via selectively varying the inclusions physical and geometrical properties, we show how one can ultra-fine and fine-tune the resonant frequency of the ADF.

  6. Correlated anomalous phase diffusion of sideband-excited phonons in an electromechanical resonator

    NASA Astrophysics Data System (ADS)

    Dong, Xiaoshi; Sun, Fengpei; Zou, Jie; Dykman, Mark; Chan, Hobun

    We study the phase fluctuations of self-sustained oscillations induced by dynamical backaction in a micromechanical resonator. The resonatorhas two vibrational modes with strongly differing frequencies and decay rates. The high-frequency mode acts as a phonon cavity mode, playing a similar role as photon modes in optomechanical systems. When sufficiently strong pumping is applied at the blue-detuned sideband of the cavity, the dynamical backaction leads to a parametric instability accompanied by self-sustained oscillations. We find that self-sustained oscillations are induced not only in the low frequency mechanical mode, but also in the high frequency cavity mode. The nonlinear nature of the backaction leads to hysteresis of this self-sustained oscillations. In each mode, the phase undergoes anomalous diffusion, where the mean square phase change in time follows a superlinear power law. The exponent of this power law is determined by the 1/f-type intrinsic frequency noise of the resonator. Remarkably, the phase fluctuation of the two modes show near perfect anti-correlation, our findings show that self-sustained oscillations induced by dynamical backaction offer new opportunities of phase manipulation and investigation of fundamental properties of resonating.

  7. Anharmonicity in light scattering by optical phonons in GaAs1-xBix

    NASA Astrophysics Data System (ADS)

    Joshya, R. S.; Rajaji, V.; Narayana, Chandrabhas; Mascarenhas, A.; Kini, R. N.

    2016-05-01

    We present a Raman spectroscopic study of GaAs1-xBix epilayers grown by molecular beam epitaxy. We have investigated the anharmonic effect on the GaAs-like longitudinal optical phonon mode ( LOGaAs' ) of GaAs1-xBix for different Bi concentrations at various temperatures. The results are analyzed in terms of the anharmonic damping effect induced by thermal and compositional disorder. We have observed that the anharmonicity increases with Bi concentration in GaAs1-xBix as evident from the increase in the anharmonicity constants. In addition, the anharmonic lifetime of the optical phonon decreases with increasing Bi concentration in GaAs1-xBix.

  8. In-situ optical transmission electron microscope study of exciton phonon replicas in ZnO nanowires by cathodoluminescence

    SciTech Connect

    Yang, Shize; Tian, Xuezeng; Wang, Lifen; Wei, Jiake; Qi, Kuo; Li, Xiaomin; Xu, Zhi E-mail: xdbai@iphy.ac.cn Wang, Wenlong; Zhao, Jimin; Bai, Xuedong E-mail: xdbai@iphy.ac.cn; Wang, Enge E-mail: xdbai@iphy.ac.cn

    2014-08-18

    The cathodoluminescence spectrum of single zinc oxide (ZnO) nanowires is measured by in-situ optical Transmission Electron Microscope. The coupling between exciton and longitudinal optical phonon is studied. The band edge emission varies for different excitation spots. This effect is attributed to the exciton propagation along the c axis of the nanowire. Contrary to free exciton emission, the phonon replicas are well confined in ZnO nanowire. They travel along the c axis and emit at the end surface. Bending strain increases the relative intensity of second order phonon replicas when excitons travel along the c-axis.

  9. Strong Coupling between Nanoscale Metamaterials and Phonons

    SciTech Connect

    Shelton, David J.; Brener, Igal; Ginn, James C.; Sinclair, Michael B.; Peters, David W.; Coffey, Kevin R.; Boreman, Glenn D.

    2011-05-11

    We use split ring resonators (SRRs) at optical frequencies to study strong coupling between planar metamaterials and phonon vibrations in nanometer-scale dielectric layers. A series of SRR metamaterials were fabricated on a semiconductor wafer with a thin intervening SiO{sub 2} dielectric layer. The dimensions of the SRRs were varied to tune the fundamental metamaterial resonance across the infrared (IR) active phonon band of SiO{sub 2} at 130 meV (31 THz). Strong anticrossing of these resonances was observed, indicative of strong coupling between metamaterial and phonon excitations. This coupling is very general and can occur with any electrically polarizable resonance including phonon vibrations in other thin film materials and semiconductor band-to-band transitions in the near to far IR. These effects may be exploited to reduce loss and to create unique spectral features that are not possible with metamaterials alone.

  10. Raman investigation of optical phonons in the ion implanted Hg1-xCdxTe

    NASA Astrophysics Data System (ADS)

    Singh, Anand; Shukla, A. K.; Pal, R.

    2016-07-01

    Raman scattering is studied here for Hg1-xCdxTe (x = 0.3) samples implanted with 180-keV of B11 ions with various doses up to 1 × 1015 cm-2. Considering disorder in the implanted HgCdTe material, the correlation length of Raman active optical phonons is determined as a short range order in the nanocrystals. Phonon softening and asymmetric broadening are investigated for HgTe like LO and TO phonon modes in the Raman spectrum while CdTe like modes almost disappeared for the dose greater than 5 × 1013 cm-2. Disorder is measured quantitatively for wide ranges of doses on the basis of phonon confinement model. Nanostructures of the near-surface implantation-induced damage layer are known to consist of a mixture of amorphous HgCdTe and its nanocrystals. A significant reduction of the nanocrystallites size is reported here with increasing dose i.e. L = 34-46 A0 at dose of 1 × 1015 cm-2.

  11. Ab initio phonon coupling and optical response of hot electrons in plasmonic metals

    NASA Astrophysics Data System (ADS)

    Brown, Ana M.; Sundararaman, Ravishankar; Narang, Prineha; Goddard, William A.; Atwater, Harry A.

    2016-08-01

    Ultrafast laser measurements probe the nonequilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics, but a parameter-free description of pump-probe measurements has not yet been possible, despite intensive research, because of the phenomenological treatment of electron-phonon interactions. We present ab initio predictions of the electron-temperature dependent heat capacities and electron-phonon coupling coefficients of plasmonic metals. We find substantial differences from free-electron and semiempirical estimates, especially in noble metals above transient electron temperatures of 2000 K, because of the previously neglected strong dependence of electron-phonon matrix elements on electron energy. We also present first-principles calculations of the electron-temperature dependent dielectric response of hot electrons in plasmonic metals, including direct interband and phonon-assisted intraband transitions, facilitating complete theoretical predictions of the time-resolved optical probe signatures in ultrafast laser experiments.

  12. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi (M =Ir , Os )

    NASA Astrophysics Data System (ADS)

    Delaire, O.; Al-Qasir, I. I.; May, A. F.; Li, C. W.; Sales, B. C.; Niedziela, J. L.; Ma, J.; Matsuda, M.; Abernathy, D. L.; Berlijn, T.

    2015-03-01

    The vibrational behavior of heavy substitutional impurities (M = Ir,Os) in Fe1-xMxSi (x =0 ,0.02 ,0.04 ,0.1 ) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. Our INS measurements on single crystals mapped the four-dimensional dynamical structure factor, S (Q ,E ) , for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers, leads to softened interatomic force constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S (Q ,E ) from INS through a Green's-function model incorporating the phonon self-energy based on first-principles density functional theory simulations, and we study the disorder-induced lifetimes on large supercells. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.

  13. High-Q cross-plate phononic crystal resonator for enhanced acoustic wave localization and energy harvesting

    NASA Astrophysics Data System (ADS)

    Yang, Aichao; Li, Ping; Wen, Yumei; Yang, Chao; Wang, Decai; Zhang, Feng; Zhang, Jiajia

    2015-05-01

    A high-Q cross-plate phononic crystal resonator (Cr-PCR) coupled with an electromechanical Helmholtz resonator (EMHR) is proposed to improve acoustic wave localization and energy harvesting. Owing to the strongly directional wave-scattering effect of the cross-plate corners, strong confinement of acoustic waves emerges. Consequently, the proposed Cr-PCR structure exhibits ∼353.5 times higher Q value and ∼6.1 times greater maximum pressure amplification than the phononic crystal resonator (Cy-PCR) (consisting of cylindrical scatterers) of the same size. Furthermore, the harvester using the proposed Cr-PCR and the EMHR has ∼22 times greater maximum output-power volume density than the previous harvester using Cy-PCR and EMHR structures.

  14. Optical phonons in nanostructured thin films composed by zincblende zinc selenide quantum dots in strong size-quantization regime: Competition between phonon confinement and strain-related effects

    SciTech Connect

    Pejova, Biljana

    2014-05-01

    Raman scattering in combination with optical spectroscopy and structural studies by X-ray diffraction was employed to investigate the phonon confinement and strain-induced effects in 3D assemblies of variable-size zincblende ZnSe quantum dots close packed in thin film form. Nanostructured thin films were synthesized by colloidal chemical approach, while tuning of the nanocrystal size was enabled by post-deposition thermal annealing treatment. In-depth insights into the factors governing the observed trends of the position and half-width of the 1LO band as a function of the average QD size were gained. The overall shifts in the position of 1LO band were found to result from an intricate compromise between the influence of phonon confinement and lattice strain-induced effects. Both contributions were quantitatively and exactly modeled. Accurate assignments of the bands due to surface optical (SO) modes as well as of the theoretically forbidden transverse optical (TO) modes were provided, on the basis of reliable physical models (such as the dielectric continuum model of Ruppin and Englman). The size-dependence of the ratio of intensities of the TO and LO modes was studied and discussed as well. Relaxation time characterizing the phonon decay processes in as-deposited samples was found to be approximately 0.38 ps, while upon post-deposition annealing already at 200 °C it increases to about 0.50 ps. Both of these values are, however, significantly smaller than those characteristic for a macrocrystalline ZnSe sample. - Graphical abstract: Optical phonons in nanostructured thin films composed by zincblende zinc selenide quantum dots in strong size-quantization regime: competition between phonon confinement and strain-related effects. - Highlights: • Phonon confinement vs. strain-induced effects in ZnSe 3D QD assemblies were studied. • Shifts of the 1LO band result from an intricate compromise between the two effects. • SO and theoretically forbidden TO modes were

  15. Surface optical phonons in GaAs nanowires grown by Ga-assisted chemical beam epitaxy

    SciTech Connect

    García Núñez, C. Braña, A. F.; Pau, J. L.; Ghita, D.; García, B. J.; Shen, G.; Wilbert, D. S.; Kim, S. M.; Kung, P.

    2014-01-21

    Surface optical (SO) phonons were studied by Raman spectroscopy in GaAs nanowires (NWs) grown by Ga-assisted chemical beam epitaxy on oxidized Si(111) substrates. NW diameters and lengths ranging between 40 and 65 nm and between 0.3 and 1.3 μm, respectively, were observed under different growth conditions. The analysis of the Raman peak shape associated to either longitudinal or surface optical modes gave important information about the crystal quality of grown NWs. Phonon confinement model was used to calculate the density of defects as a function of the NW diameter resulting in values between 0.02 and 0.03 defects/nm, indicating the high uniformity obtained on NWs cross section size during growth. SO mode shows frequency downshifting as NW diameter decreases, this shift being sensitive to NW sidewall oxidation. The wavevector necessary to activate SO phonon was used to estimate the NW facet roughness responsible for SO shift.

  16. Spin-flip relaxation via optical phonon scattering in quantum dots

    SciTech Connect

    Wang, Zi-Wu; Liu, Lei; Li, Shu-Shen

    2013-12-14

    Based on the spin-orbit coupling admixture mechanism, we theoretically investigate the spin-flip relaxation via optical phonon scattering in quantum dots by considering the effect of lattice relaxation due to the electron-acoustic phonon deformation potential coupling. The relaxation rate displays a cusp-like structure (or a spin hot spot) that becomes more clearly with increasing temperature. We also calculate the relaxation rate of the spin-conserving process, which follows a Gaussian form and is several orders of magnitude larger than that of spin-flip process. Moreover, we find that the relaxation rate displays the oscillatory behavior due to the interplay effects between the magnetic and spatial confinement for the spin-flip process not for the spin-conserving process. The trends of increasing and decreasing temperature dependence of the relaxation rates for two relaxation processes are obtained in the present model.

  17. Low-energy optical phonon modes in the caged compound LaRu2Zn20

    NASA Astrophysics Data System (ADS)

    Wakiya, K.; Onimaru, T.; Tsutsui, S.; Hasegawa, T.; Matsumoto, K. T.; Nagasawa, N.; Baron, A. Q. R.; Ogita, N.; Udagawa, M.; Takabatake, T.

    2016-02-01

    We have investigated atomic dynamics of caged compound LaRu2Zn20 by the measurements of specific heat C and inelastic x-ray scattering (IXS). The lattice part of the specific heat Clat divided by T3,Clat /T3, shows a broad peak at around 15 K, which is reproduced by two Einstein modes with characteristic temperatures of θE 1=35 K and θE 2=82 K, respectively. IXS measurements along the [111] and [110] directions reveal weakly dispersive phonon modes at 3 meV (35 K) and 7 meV (80 K), respectively, whose values agree with the values of θE's. The first-principles calculation has assigned the 3 meV phonon modes as the optical modes of Zn atoms located at the middle of two La atoms, which is likely to lead to the structural instability.

  18. Phonon sideband studies of the spin-triplet optical transition in diamond nitrogen-vacancy centers

    NASA Astrophysics Data System (ADS)

    Alkauskas, Audrius; Toyli, David M.; Buckley, Bob B.; Awschalom, David D.; van de Walle, Chris G.

    2013-03-01

    In the past decade, the nitrogen-vacancy center in diamond has emerged as a promising solid-state system for quantum-information processing, and also for nanoscale magnetic, electric, and thermal sensing. All of these applications are partly enabled because the spin of the center can be measured through photoluminescence. This calls for a deeper understanding of the photoluminescence spectrum, in particular its phonon side-band. In this work we study the coupling of lattice vibrations to the triplet (3E -->3A2) optical transition from first-principles electronic structure calculations. Our formulation includes both quasi-localized and bulk phonons, and leads to an excellent agreement of the calculated and the measured photoluminescence lineshape. This good agreement enables the application of the developed methodology to other defects in semiconductors that are currently being investigated as viable quantum bits. This work has been supported by the NSF, AFOSR, and the Swiss NSF.

  19. Decoherence dynamics of interacting qubits coupled to a bath of local optical phonons

    NASA Astrophysics Data System (ADS)

    Lone, Muzaffar Qadir; Yarlagadda, S.

    2016-04-01

    We study decoherence in an interacting qubit system described by infinite range Heisenberg model (IRHM) in a situation where the system is coupled to a bath of local optical phonons. Using perturbation theory in polaron frame of reference, we derive an effective Hamiltonian that is valid in the regime of strong spin-phonon coupling under nonadiabatic conditions. It is shown that the effective Hamiltonian commutes with the IRHM upto leading orders of perturbation and thus has the same eigenstates as the IRHM. Using a quantum master equation with Markovian approximation of dynamical evolution, we show that the off-diagonal elements of the density matrix do not decay in the energy eigen basis of IRHM.

  20. Scanning Tunneling Optical Resonance Microscopy

    NASA Technical Reports Server (NTRS)

    Bailey, Sheila; Wilt, Dave; Raffaelle, Ryne; Gennett, Tom; Tin, Padetha; Lau, Janice; Castro, Stephanie; Jenkins, Philip; Scheiman, Dave

    2003-01-01

    Scanning tunneling optical resonance microscopy (STORM) is a method, now undergoing development, for measuring optoelectronic properties of materials and devices on the nanoscale by means of a combination of (1) traditional scanning tunneling microscopy (STM) with (2) tunable laser spectroscopy. In STORM, an STM tip probing a semiconductor is illuminated with modulated light at a wavelength in the visible-to-near-infrared range and the resulting photoenhancement of the tunneling current is measured as a function of the illuminating wavelength. The photoenhancement of tunneling current occurs when the laser photon energy is sufficient to excite charge carriers into the conduction band of the semiconductor. Figure 1 schematically depicts a proposed STORM apparatus. The light for illuminating the semiconductor specimen at the STM would be generated by a ring laser that would be tunable across the wavelength range of interest. The laser beam would be chopped by an achromatic liquid-crystal modulator. A polarization-maintaining optical fiber would couple the light to the tip/sample junction of a commercial STM. An STM can be operated in one of two modes: constant height or constant current. A STORM apparatus would be operated in the constant-current mode, in which the height of the tip relative to the specimen would be varied in order to keep the tunneling current constant. In this mode, a feedback control circuit adjusts the voltage applied to a piezoelectric actuator in the STM that adjusts the height of the STM tip to keep the tunneling current constant. The exponential relationship between the tunneling current and tip-to-sample distance makes it relatively easy to implement this mode of operation. The choice of method by which the photoenhanced portion of the tunneling current would be measured depends on choice of the frequency at which the input illumination would be modulated (chopped). If the frequency of modulation were low enough (typically < 10 Hz) that the

  1. Coupled optical resonance laser locking

    NASA Astrophysics Data System (ADS)

    Burd, S. C.; du Toit, P. J. W.; Uys, H.

    2014-10-01

    We have demonstrated simultaneous laser frequency stabilization of a UV and IR laser, to the same spectroscopic sample, by monitoring only the absorption of the UV laser. For trapping and cooling Yb$^{+}$ ions, a frequency stabilized laser is required at 369.95nm to drive the $^{2}S_{1/2}$ $ \\rightarrow $ $ ^{2}P_{1/2}$ cooling transition. Since the cycle is not closed, a 935.18nm laser is needed to drive the $^{2}D_{3/2}$ $\\rightarrow$ $^{3}D_{[3/2]1/2}$ transition which is followed by rapid decay to the $^{2}S_{1/2}$ state. Our 369nm laser is locked to Yb$^{+}$ ions generated in a hollow cathode discharge lamp using saturated absorption spectroscopy. Without pumping, the metastable $^{2}D_{3/2}$ level is only sparsely populated and direct absorption of 935nm light is difficult to detect. A resonant 369nm laser is able to significantly populate the $^{2}D_{3/2}$ state due to the coupling between the levels. Fast re-pumping to the $^{2}S_{1/2}$ state, by 935nm light, can be detected by observing the change in absorption of the 369nm laser using lock-in detection of the photodiode signal. In this way simultaneous locking of two optical frequencies in very different spectral regimes is accomplished. A rate equation model gives good qualitative agreement with the experimental results. This technique offers improved laser frequency stabilization compared to lasers locked individually to the sample and should be readily applicable to similar ion systems.

  2. Coherent Control of Optically Generated and Detected Picosecond Surface Acoustic Phonons

    SciTech Connect

    David H. Hurley

    2006-11-01

    Coherent control of elementary optical excitations is a key issue in ultrafast materials science. Manipulation of electronic and vibronic excitations in solids as well as chemical and biological systems on ultrafast time scales has attracted a great deal of attention recently. In semiconductors, coherent control of vibronic excitations has been demonstrated for bulk acoustic and optical phonons generated in superlattice structures. The bandwidth of these approaches is typically fully utilized by employing a 1-D geometry where the laser spot size is much larger than the superlattice repeat length. In this presentation we demonstrate coherent control of optically generated picosecond surface acoustic waves using sub-optical wavelength absorption gratings. The generation and detection characteristics of two material systems are investigated (aluminum absorption gratings on Si and GaAs substrates).

  3. Fermi resonance in optical microcavities

    NASA Astrophysics Data System (ADS)

    Yi, Chang-Hwan; Yu, Hyeon-Hye; Lee, Ji-Won; Kim, Chil-Min

    2015-04-01

    Fermi resonance is a phenomenon of quantum mechanical superposition, which most often occurs between normal and overtone modes in molecular systems that are nearly coincident in energy. We find that scarred resonances in deformed dielectric microcavities are the very phenomenon of Fermi resonance, that is, a pair of quasinormal modes interact with each other due to coupling and a pair of resonances are generated through an avoided resonance crossing. Then the quantum number difference of a pair of quasinormal modes, which is a consequence of quantum mechanical superposition, equals periodic orbits, whereby the resonances are localized on the periodic orbits. We derive the relation between the quantum number difference and the periodic orbits and confirm it in an elliptic, a rectangular, and a stadium-shaped dielectric microcavity.

  4. Direct measurement of lattice dynamics and optical phonon excitation in semiconductor nanocrystals using femtosecond stimulated Raman spectroscopy.

    PubMed

    Hannah, Daniel C; Brown, Kristen E; Young, Ryan M; Wasielewski, Michael R; Schatz, George C; Co, Dick T; Schaller, Richard D

    2013-09-01

    We report femtosecond stimulated Raman spectroscopy measurements of lattice dynamics in semiconductor nanocrystals and characterize longitudinal optical (LO) phonon production during confinement-enhanced, ultrafast intraband relaxation. Stimulated Raman signals from unexcited CdSe nanocrystals produce a spectral shape similar to spontaneous Raman signals. Upon photoexcitation, stimulated Raman amplitude decreases owing to experimentally resolved ultrafast phonon generation rates within the lattice. We find a ∼600  fs, particle-size-independent depletion time attributed to hole cooling, evidence of LO-to-acoustic down-conversion, and LO phonon mode softening. PMID:25166708

  5. Real-space transfer of photoexcited electrons in type-II superlattices via optical-phonon emission

    SciTech Connect

    Erdogan, M.U.; Sankaran, V.; Kim, K.W.; Stroscio, M.A.; Iafrate, G.J.

    1994-12-31

    The {Gamma}-{Chi} scattering rate of electron is type-II superlattices by optical-phonon emission is calculated. The tight binding method for electronic band structure and the dielectric continuum model for phonons are used. The relative strength of scattering due to different phonon modes is examined for varying superlattice dimensions. The scattering rate is highest when the energy separation between the {Gamma} and {Chi} levels is smallest, and decreases quickly as the separation increases. It is found that the strongest scattering rate is due to the emission of AlAs confined modes. Changing of parity with layer thickness and its effect on scattering are discussed.

  6. Axial interface optical phonon modes in a double-nanoshell system.

    PubMed

    Kanyinda-Malu, C; Clares, F J; de la Cruz, R M

    2008-07-16

    Within the framework of the dielectric continuum (DC) model, we analyze the axial interface optical phonon modes in a double system of nanoshells. This system is constituted by two identical equidistant nanoshells which are embedded in an insulating medium. To illustrate our results, typical II-VI semiconductors are used as constitutive polar materials of the nanoshells. Resolution of Laplace's equation in bispherical coordinates for the potentials derived from the interface vibration modes is made. By imposing the usual electrostatic boundary conditions at the surfaces of the two-nanoshell system, recursion relations for the coefficients appearing in the potentials are obtained, which entails infinite matrices. The problem of deriving the interface frequencies is reduced to the eigenvalue problem on infinite matrices. A truncating method for these matrices is used to obtain the interface phonon branches. Dependences of the interface frequencies on the ratio of inter-nanoshell separation to core size are obtained for different systems with several values of nanoshell interdistance. Effects due to the change of shell and embedding materials are also investigated in interface phonon modes. PMID:21828747

  7. Ultra-high frequency, high Q/volume micromechanical resonators in a planar AlN phononic crystal

    NASA Astrophysics Data System (ADS)

    Ghasemi Baboly, M.; Alaie, S.; Reinke, C. M.; El-Kady, I.; Leseman, Z. C.

    2016-07-01

    This paper presents the first design and experimental demonstration of an ultrahigh frequency complete phononic crystal (PnC) bandgap aluminum nitride (AlN)/air structure operating in the GHz range. A complete phononic bandgap of this design is used to efficiently and simultaneously confine elastic vibrations in a resonator. The PnC structure is fabricated by etching a square array of air holes in an AlN slab. The fabricated PnC resonator resonates at 1.117 GHz, which corresponds to an out-of-plane mode. The measured bandgap and resonance frequencies are in very good agreement with the eigen-frequency and frequency-domain finite element analyses. As a result, a quality factor/volume of 7.6 × 1017/m3 for the confined resonance mode was obtained that is the largest value reported for this type of PnC resonator to date. These results are an important step forward in achieving possible applications of PnCs for RF communication and signal processing with smaller dimensions.

  8. Phonon effects on x-ray absorption and nuclear magnetic resonance spectroscopies

    NASA Astrophysics Data System (ADS)

    Nemausat, Ruidy; Cabaret, Delphine; Gervais, Christel; Brouder, Christian; Trcera, Nicolas; Bordage, Amélie; Errea, Ion; Mauri, Francesco

    2015-10-01

    In material sciences, spectroscopic approaches combining ab initio calculations with experiments are commonly used to accurately analyze the experimental spectral data. Most state-of-the-art first-principles calculations are usually performed assuming an equilibrium static lattice. Yet, nuclear motion affects spectra even when reduced to the zero-point motion at 0 K. We propose a framework based on density-functional theory that includes quantum thermal fluctuations in theoretical x-ray absorption near-edge structure (XANES) and solid-state nuclear magnetic resonance (NMR) spectroscopies and allows to well describe temperature effects observed experimentally. Within the Born-Oppenheimer and quasiharmonic approximations, we incorporate the nuclear motion by generating several nonequilibrium configurations from the dynamical matrix. The averaged calculated XANES and NMR spectral data have been compared to experiments in MgO. The good agreement obtained between experiments and calculations validates the developed approach, which suggests that calculating the XANES spectra at finite temperature by averaging individual nonequilibrium configurations is a suitable approximation. This study highlights the relevance of phonon renormalization and the relative contributions of thermal expansion and nuclear dynamics on NMR and XANES spectra on a wide range of temperatures.

  9. Phonon Cooling by an Optomechanical Heat Pump

    NASA Astrophysics Data System (ADS)

    Dong, Ying; Bariani, F.; Meystre, P.

    2015-11-01

    We propose and analyze theoretically a cavity optomechanical analog of a heat pump that uses a polariton fluid to cool mechanical modes coupled to a single precooled phonon mode via external modulation of the substrate of the mechanical resonator. This approach permits us to cool phonon modes of arbitrary frequencies not limited by the cavity-optical field detuning deep into the quantum regime from room temperature.

  10. Resonance spectra of diabolo optical antenna arrays

    NASA Astrophysics Data System (ADS)

    Guo, Hong; Simpkins, Blake; Caldwell, Joshua D.; Guo, Junpeng

    2015-10-01

    A complete set of diabolo optical antenna arrays with different waist widths and periods was fabricated on a sapphire substrate by using a standard e-beam lithography and lift-off process. Fabricated diabolo optical antenna arrays were characterized by measuring the transmittance and reflectance with a microscope-coupled FTIR spectrometer. It was found experimentally that reducing the waist width significantly shifts the resonance to longer wavelength and narrowing the waist of the antennas is more effective than increasing the period of the array for tuning the resonance wavelength. Also it is found that the magnetic field enhancement near the antenna waist is correlated to the shift of the resonance wavelength.

  11. Resonance spectra of diabolo optical antenna arrays

    SciTech Connect

    Guo, Hong; Guo, Junpeng; Simpkins, Blake; Caldwell, Joshua D.

    2015-10-15

    A complete set of diabolo optical antenna arrays with different waist widths and periods was fabricated on a sapphire substrate by using a standard e-beam lithography and lift-off process. Fabricated diabolo optical antenna arrays were characterized by measuring the transmittance and reflectance with a microscope-coupled FTIR spectrometer. It was found experimentally that reducing the waist width significantly shifts the resonance to longer wavelength and narrowing the waist of the antennas is more effective than increasing the period of the array for tuning the resonance wavelength. Also it is found that the magnetic field enhancement near the antenna waist is correlated to the shift of the resonance wavelength.

  12. Optical properties of Eu3+-doped antimony-oxide-based low phonon disordered matrices

    NASA Astrophysics Data System (ADS)

    Som, Tirtha; Karmakar, Basudeb

    2010-01-01

    A new series of monolithic Eu2O3-doped high antimony oxide (40-80 mol%) content disordered matrices (glasses) of low phonon energy (about 600 cm-1) in the K2O-B2O3-Sb2O3 (KBS) system was prepared by the melt-quench technique. Infrared reflection spectroscopy was used to establish the low phonon energy of the glasses. Amorphicity and devitrification of the glasses were confirmed by x-ray diffraction analysis. UV-vis absorption spectra of Eu3+ have been measured and the band positions have been justified with quantitative calculation of the nephelauxetic parameter and covalent bonding characteristics of the host. These Eu2O3-doped glasses upon excitation at 393 nm radiation exhibit six emission bands in the range 500-750 nm due to their low phonon energy. Of these, the magnetic dipole ^{5}\\mathrm {D}_{0} \\to {}^{7} \\mathrm {F_{1}} transition shows small Stark splitting while the electric dipole ^{5}\\mathrm {D}_{0} \\to {}^{7}\\mathrm {F}_{2} transition undergoes remarkable Stark splitting into two components. They have been explained by the crystal field effect. The Judd-Ofelt parameters, Ωt = 2,4,6, were also evaluated and the change of Ωt with the glass composition was correlated with the asymmetric effect at Eu3+ ion sites and the fundamental properties like covalent character and optical basicity. We are the first to report the spectroscopic properties of the Eu3+ ion in KBS low phonon antimony glasses.

  13. Method of shifting and fixing optical frequency of an optical resonator, and optical resonator made by same

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy A. (Inventor); Strekalov, Dmitry V. (Inventor); Maleki, Lute (Inventor); Matsko, Andrey B. (Inventor); Iltchenko, Vladimir S. (Inventor); Martin, Jan M. (Inventor)

    2010-01-01

    A method of shifting and fixing an optical frequency of an optical resonator to a desired optical frequency, and an optical resonator made by such a method are provided. The method includes providing an optical resonator having a surface and a refractive index, and obtaining a coating composition having a predetermined concentration of a substance and having a refractive index that is substantially similar to the refractive index of the optical resonator. The coating composition inherently possesses a thickness when it is applied as a coating. The method further includes determining a coating ratio for the surface of the optical resonator and applying the coating composition onto a portion of the surface of the optical resonator based upon the determined coating ratio.

  14. Electric-optic resonant phase modulator

    NASA Technical Reports Server (NTRS)

    Chen, Chien-Chung (Inventor); Robinson, Deborah L. (Inventor); Hemmati, Hamid (Inventor)

    1994-01-01

    An electro-optic resonant cavity is used to achieve phase modulation with lower driving voltages. Laser damage thresholds are inherently higher than with previously used integrated optics due to the utilization of bulk optics. Phase modulation is achieved at higher speeds with lower driving voltages than previously obtained with non-resonant electro-optic phase modulators. The instant scheme uses a data locking dither approach as opposed to the conventional sinusoidal locking schemes. In accordance with a disclosed embodiment, a resonant cavity modulator has been designed to operate at a data rate in excess of 100 Mbps. By carefully choosing the cavity finesse and its dimension, it is possible to control the pulse switching time to within 4 ns and to limit the required switching voltage to within 10 V. Experimentally, the resonant cavity can be maintained on resonance with respect to the input laser signal by monitoring the fluctuation of output intensity as the cavity is switched. This cavity locking scheme can be applied by using only the random data sequence, and without the need of additional dithering of the cavity. Compared to waveguide modulators, the resonant cavity has a comparable modulating voltage requirement. Because of its bulk geometry, resonant cavity modulator has the potential of accommodating higher throughput power. Furthermore, mode matching into a bulk device is easier and typically can be achieved with higher efficiency. On the other hand, unlike waveguide modulators which are essentially traveling wave devices, the resonant cavity modulator requires that the cavity be maintained in resonance with respect to the incoming laser signal. An additional control loop is incorporated into the modulator to maintain the cavity on resonance.

  15. Unified Description of the Optical Phonon Modes in N-Layer MoTe2.

    PubMed

    Froehlicher, Guillaume; Lorchat, Etienne; Fernique, François; Joshi, Chaitanya; Molina-Sánchez, Alejandro; Wirtz, Ludger; Berciaud, Stéphane

    2015-10-14

    N-layer transition metal dichalcogenides provide a unique platform to investigate the evolution of the physical properties between the bulk (three-dimensional) and monolayer (quasi-two-dimensional) limits. Here, using high-resolution micro-Raman spectroscopy, we report a unified experimental description of the Γ-point optical phonons in N-layer 2H-molybdenum ditelluride (MoTe2). We observe series of N-dependent low-frequency interlayer shear and breathing modes (below 40 cm(-1), denoted LSM and LBM) and well-defined Davydov splittings of the mid-frequency modes (in the range 100-200 cm(-1), denoted iX and oX), which solely involve displacements of the chalcogen atoms. In contrast, the high-frequency modes (in the range 200-300 cm(-1), denoted iMX and oMX), arising from displacements of both the metal and chalcogen atoms, exhibit considerably reduced splittings. The manifold of phonon modes associated with the in-plane and out-of-plane displacements are quantitatively described by a force constant model, including interactions up to the second nearest neighbor and surface effects as fitting parameters. The splittings for the iX and oX modes observed in N-layer crystals are directly correlated to the corresponding bulk Davydov splittings between the E2u/E1g and B1u/A1g modes, respectively, and provide a measurement of the frequencies of the bulk silent E2u and B1u optical phonon modes. Our analysis could readily be generalized to other layered crystals. PMID:26371970

  16. Electro-optic resonant phase modulator

    NASA Technical Reports Server (NTRS)

    Chen, Chien-Chung (Inventor); Hemmati, Hamid (Inventor); Robinson, Deborah L. (Inventor)

    1992-01-01

    An electro-optic resonant cavity is used to achieve phase modulation with lower driving voltages. Laser damage thresholds are inherently higher than with previously used integrated optics due to the utilization of bulk optics. Phase modulation is achieved at higher speeds with lower driving voltages than previously obtained with non-resonant electro-optic phase modulators. The instant scheme uses a data locking dither approach as opposed to the conventional sinusoidal locking schemes. In accordance with a disclosed embodiment, a resonant cavity modulator has been designed to operate at a data rate in excess of 100 megabits per sec. By carefully choosing the cavity finesse and its dimension, it is possible to control the pulse switching time to within 4 nano-sec. and to limit the required switching voltage to within 10 V. This cavity locking scheme can be applied by using only the random data sequence, and without the need of dithering of the cavity. Compared to waveguide modulators, the resonant cavity has a comparable modulating voltage requirement. Because of its bulk geometry, the resonant cavity modulator has the potential of accommodating higher throughput power. Mode matching into the bulk device is easier and typically can be achieved with higher efficiency. An additional control loop is incorporated into the modulator to maintain the cavity on resonance.

  17. Terahertz instability of surface optical-phonon polaritons that interact with surface plasmon polaritons in the presence of electron drift

    SciTech Connect

    Sydoruk, O.; Solymar, L.; Shamonina, E.; Kalinin, V.

    2010-10-15

    Traveling-wave interaction between optical phonons and electrons drifting in diatomic semiconductors has potential for amplification and generation of terahertz radiation. Existing models of this interaction were developed for infinite materials. As a more practically relevant configuration, we studied theoretically a finite semiconductor slab surrounded by a dielectric. This paper analyzes the optical-phonon instability in the slab including the Lorentz force and compares it to the instability in an infinite material. As the analysis shows, the slab instability occurs because of the interaction of surface optical-phonon polaritons with surface plasmon polaritons in the presence of electron drift. The properties of the instability depend on the slab thickness when the thickness is comparable to the wavelength. For large slab thicknesses, however, the dispersion relation of the slab is similar to that of an infinite material, although the coupling is weaker. The results could be used for the design of practical terahertz traveling-wave oscillators and amplifiers.

  18. p -State Luminescence in CdSe Nanoplatelets: Role of Lateral Confinement and a Longitudinal Optical Phonon Bottleneck

    NASA Astrophysics Data System (ADS)

    Achtstein, Alexander W.; Scott, Riccardo; Kickhöfel, Sebastian; Jagsch, Stefan T.; Christodoulou, Sotirios; Bertrand, Guillaume H. V.; Prudnikau, Anatol V.; Antanovich, Artsiom; Artemyev, Mikhail; Moreels, Iwan; Schliwa, Andrei; Woggon, Ulrike

    2016-03-01

    We evidence excited state emission from p states well below ground state saturation in CdSe nanoplatelets. Size-dependent exciton ground and excited state energies and population dynamics are determined by four independent methods: time-resolved PL, time-integrated PL, rate equation modeling, and Hartree renormalized k .p calculations—all in very good agreement. The ground state-excited state energy spacing strongly increases with the lateral platelet quantization. Depending on its detuning to the LO phonon energy, the PL decay of CdSe platelets is governed by a size tunable LO phonon bottleneck, related to the low exciton-phonon coupling, very large oscillator strength, and energy spacing of both states. This is, for instance, ideal to tune lasing properties. CdSe platelets are perfectly suited to control the exciton-phonon interaction by changing their lateral size while the optical transition energy is determined by their thickness.

  19. p-State Luminescence in CdSe Nanoplatelets: Role of Lateral Confinement and a Longitudinal Optical Phonon Bottleneck.

    PubMed

    Achtstein, Alexander W; Scott, Riccardo; Kickhöfel, Sebastian; Jagsch, Stefan T; Christodoulou, Sotirios; Bertrand, Guillaume H V; Prudnikau, Anatol V; Antanovich, Artsiom; Artemyev, Mikhail; Moreels, Iwan; Schliwa, Andrei; Woggon, Ulrike

    2016-03-18

    We evidence excited state emission from p states well below ground state saturation in CdSe nanoplatelets. Size-dependent exciton ground and excited state energies and population dynamics are determined by four independent methods: time-resolved PL, time-integrated PL, rate equation modeling, and Hartree renormalized k·p calculations-all in very good agreement. The ground state-excited state energy spacing strongly increases with the lateral platelet quantization. Depending on its detuning to the LO phonon energy, the PL decay of CdSe platelets is governed by a size tunable LO phonon bottleneck, related to the low exciton-phonon coupling, very large oscillator strength, and energy spacing of both states. This is, for instance, ideal to tune lasing properties. CdSe platelets are perfectly suited to control the exciton-phonon interaction by changing their lateral size while the optical transition energy is determined by their thickness. PMID:27035317

  20. Transport coefficients of graphene: Interplay of impurity scattering, Coulomb interaction, and optical phonons

    NASA Astrophysics Data System (ADS)

    Xie, Hong-Yi; Foster, Matthew S.

    2016-05-01

    We study the electric and thermal transport of the Dirac carriers in monolayer graphene using the Boltzmann-equation approach. Motivated by recent thermopower measurements [F. Ghahari, H.-Y. Xie, T. Taniguchi, K. Watanabe, M. S. Foster, and P. Kim, Phys. Rev. Lett. 116, 136802 (2016), 10.1103/PhysRevLett.116.136802], we consider the effects of quenched disorder, Coulomb interactions, and electron-optical-phonon scattering. Via an unbiased numerical solution to the Boltzmann equation we calculate the electrical conductivity, thermopower, and electronic component of the thermal conductivity, and discuss the validity of Mott's formula and of the Wiedemann-Franz law. An analytical solution for the disorder-only case shows that screened Coulomb impurity scattering, although elastic, violates the Wiedemann-Franz law even at low temperature. For the combination of carrier-carrier Coulomb and short-ranged impurity scattering, we observe the crossover from the interaction-limited (hydrodynamic) regime to the disorder-limited (Fermi-liquid) regime. In the former, the thermopower and the thermal conductivity follow the results anticipated by the relativistic hydrodynamic theory. On the other hand, we find that optical phonons become non-negligible at relatively low temperatures and that the induced electron thermopower violates Mott's formula. Combining all of these scattering mechanisms, we obtain the thermopower that quantitatively coincides with the experimental data.

  1. Measurement of the acoustic-to-optical phonon coupling in multicomponent systems

    NASA Astrophysics Data System (ADS)

    Caretta, Antonio; Donker, Michiel C.; Perdok, Diederik W.; Abbaszadeh, Davood; Polyakov, Alexey O.; Havenith, Remco W. A.; Palstra, Thomas T. M.; van Loosdrecht, Paul H. M.

    2015-02-01

    In this paper we investigate the acoustic-to-optical up-conversion phonon processes in a multicomponent system. These processes take place during heat transport and limit the efficiency of heat flow. By combining time-resolved optical and heat capacity experiments we quantify the thermal coupling constant to be g ˜0.4 1017 W/Km3 . The method is based on selective excitation of a part of a multicomponent system, and the measurement of the thermalization dynamics by probing the linear birefringence of the sample with femtosecond resolution. In particular, we study a layered multiferroic organic-inorganic hybrid, in the vicinity of the ferroelectric phase transition. A diverging term of the heat capacity is associated to soft-mode dynamics, in agreement with previous spectroscopy measurements.

  2. Optical and phonon properties of ZnO:CuO mixed nanocomposite

    SciTech Connect

    Udayabhaskar, R.; Karthikeyan, B.

    2014-04-21

    Optical and phonon properties of ZnO:CuO nanocrystals which are prepared through sol-gel method are reported here. From X-ray diffraction studies, observed that Cu doping replaces the Zn and also forms secondary phase. Optical absorption spectral studies shows that the exciton and plasmon related bands of ZnO and CuO phase, respectively. Fluorescence studies of the prepared samples shows that green emission from ZnO is completely depleted and the same is attributed to CuO Plasmon. Raman spectral studies reveal that secondary phase (impurity) induced profile changes in 1LO and E{sub 2High} modes. Asymmetry in peak shape is analyzed using Fano profile with the combination of Lorentzian profile. Moreover, the monotonic increase of Fano factor and full width at half maxima is hopefully attributed to the continuum arises by the plasmons of Cu-O phase in ZnO nanosystem.

  3. Optical and phonon properties of ZnO:CuO mixed nanocomposite

    NASA Astrophysics Data System (ADS)

    Udayabhaskar, R.; Karthikeyan, B.

    2014-04-01

    Optical and phonon properties of ZnO:CuO nanocrystals which are prepared through sol-gel method are reported here. From X-ray diffraction studies, observed that Cu doping replaces the Zn and also forms secondary phase. Optical absorption spectral studies shows that the exciton and plasmon related bands of ZnO and CuO phase, respectively. Fluorescence studies of the prepared samples shows that green emission from ZnO is completely depleted and the same is attributed to CuO Plasmon. Raman spectral studies reveal that secondary phase (impurity) induced profile changes in 1LO and E2High modes. Asymmetry in peak shape is analyzed using Fano profile with the combination of Lorentzian profile. Moreover, the monotonic increase of Fano factor and full width at half maxima is hopefully attributed to the continuum arises by the plasmons of Cu-O phase in ZnO nanosystem.

  4. The hydrogen-bond network of water supports propagating optical phonon-like modes.

    PubMed

    Elton, Daniel C; Fernández-Serra, Marivi

    2016-01-01

    The local structure of liquid water as a function of temperature is a source of intense research. This structure is intimately linked to the dynamics of water molecules, which can be measured using Raman and infrared spectroscopies. The assignment of spectral peaks depends on whether they are collective modes or single-molecule motions. Vibrational modes in liquids are usually considered to be associated to the motions of single molecules or small clusters. Using molecular dynamics simulations, here we find dispersive optical phonon-like modes in the librational and OH-stretching bands. We argue that on subpicosecond time scales these modes propagate through water's hydrogen-bond network over distances of up to 2 nm. In the long wavelength limit these optical modes exhibit longitudinal-transverse splitting, indicating the presence of coherent long-range dipole-dipole interactions, as in ice. Our results indicate the dynamics of liquid water have more similarities to ice than previously thought. PMID:26725363

  5. Quasi-monolithic tunable optical resonator

    NASA Technical Reports Server (NTRS)

    Arbore, Mark (Inventor); Tapos, Francisc (Inventor)

    2003-01-01

    An optical resonator has a piezoelectric element attached to a quasi-monolithic structure. The quasi-monolithic structure defines an optical path. Mirrors attached to the structure deflect light along the optical path. The piezoelectric element controllably strains the quasi-monolithic structure to change a length of the optical path by about 1 micron. A first feedback loop coupled to the piezoelectric element provides fine control over the cavity length. The resonator may include a thermally actuated spacer attached to the cavity and a mirror attached to the spacer. The thermally actuated spacer adjusts the cavity length by up to about 20 microns. A second feedback loop coupled to the sensor and heater provides a coarse control over the cavity length. An alternative embodiment provides a quasi-monolithic optical parametric oscillator (OPO). This embodiment includes a non-linear optical element within the resonator cavity along the optical path. Such an OPO configuration is broadly tunable and capable of mode-hop free operation for periods of 24 hours or more.

  6. Tunable Optical Filters Having Electro-optic Whispering-gallery-mode Resonators

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy (Inventor); Ilchenko, Vladimir (Inventor); Matsko, Andrey B. (Inventor); Maleki, Lutfollah (Inventor)

    2006-01-01

    Tunable optical filters using whispering-gallery-mode (WGM) optical resonators are described. The WGM optical resonator in a filter exhibits an electro-optical effect and hence is tunable by applying a control electrical signal.

  7. Optical isolation via unidirectional resonant photon tunneling

    SciTech Connect

    Moccia, Massimo; Castaldi, Giuseppe; Galdi, Vincenzo; Alù, Andrea; Engheta, Nader

    2014-01-28

    We show that tri-layer structures combining epsilon-negative and magneto-optical material layers can exhibit unidirectional resonant photon tunneling phenomena that can discriminate between circularly polarized (CP) waves of given handedness impinging from opposite directions, or between CP waves with different handedness impinging from the same direction. This physical principle, which can also be interpreted in terms of a Fabry-Perot-type resonance, may be utilized to design compact optical isolators for CP waves. Within this framework, we derive simple analytical conditions and design formulae, and quantitatively assess the isolation performance, also taking into account the unavoidable imperfections and nonidealities.

  8. Optically selective, acoustically resonant gas detecting transducer

    NASA Technical Reports Server (NTRS)

    Dimeff, J. (Inventor)

    1977-01-01

    A gas analyzer is disclosed which responds to the resonant absorption or emission spectrum of a specific gas by producing an acoustic resonance in a chamber containing a sample of that gas, and which measures the amount of that emission or absorption by measuring the strength of that acoustic resonance, e.g., the maximum periodic pressure, velocity or density achieved. In the preferred embodiment, a light beam is modulated periodically at the acoustical resonance frequency of a closed chamber which contains an optically dense sample of the gas of interest. Periodic heating of the absorbing gas by the light beam causes a cyclic expansion, movement, and pressure within the gas. An amplitude is reached where the increased losses were the cyclic radiation energy received. A transducing system is inclined for converting the pressure variations of the resonant gas into electronic readout signals.

  9. Chemical Sensors Based on Optical Ring Resonators

    NASA Technical Reports Server (NTRS)

    Homer, Margie; Manfreda, Allison; Mansour, Kamjou; Lin, Ying; Ksendzov, Alexander

    2005-01-01

    Chemical sensors based on optical ring resonators are undergoing development. A ring resonator according to this concept is a closed-circuit dielectric optical waveguide. The outermost layer of this waveguide, analogous to the optical cladding layer on an optical fiber, is a made of a polymer that (1) has an index of refraction lower than that of the waveguide core and (2) absorbs chemicals from the surrounding air. The index of refraction of the polymer changes with the concentration of absorbed chemical( s). The resonator is designed to operate with relatively strong evanescent-wave coupling between the outer polymer layer and the electromagnetic field propagating along the waveguide core. By virtue of this coupling, the chemically induced change in index of refraction of the polymer causes a measurable shift in the resonance peaks of the ring. In a prototype that has been used to demonstrate the feasibility of this sensor concept, the ring resonator is a dielectric optical waveguide laid out along a closed path resembling a racetrack (see Figure 1). The prototype was fabricated on a silicon substrate by use of standard techniques of thermal oxidation, chemical vapor deposition, photolithography, etching, and spin coating. The prototype resonator waveguide features an inner cladding of SiO2, a core of SixNy, and a chemical-sensing outer cladding of ethyl cellulose. In addition to the ring Chemical sensors based on optical ring resonators are undergoing development. A ring resonator according to this concept is a closed-circuit dielectric optical waveguide. The outermost layer of this waveguide, analogous to the optical cladding layer on an optical fiber, is a made of a polymer that (1) has an index of refraction lower than that of the waveguide core and (2) absorbs chemicals from the surrounding air. The index of refraction of the polymer changes with the concentration of absorbed chemical( s). The resonator is designed to operate with relatively strong

  10. Hot-electron cooling by acoustic and optical phonons in monolayers of MoS2 and other transition-metal dichalcogenides

    NASA Astrophysics Data System (ADS)

    Kaasbjerg, Kristen; Bhargavi, K. S.; Kubakaddi, S. S.

    2014-10-01

    We study hot-electron cooling by acoustic and optical phonons in monolayer MoS2. The cooling power P (Pe=P /n ) is investigated as a function of electron temperature Te (0-500 K) and carrier density n (1010-1013 cm-2) taking into account all relevant electron-phonon (el-ph) couplings. We find that the crossover from acoustic phonon dominated cooling at low Te to optical phonon dominated cooling at higher Te takes place at Te˜50 -75 K. The unscreened deformation potential (DP) coupling to the TA phonon is shown to dominate P due to acoustic phonon scattering over the entire temperature and density range considered. The cooling power due to screened DP coupling to the LA phonon and screened piezoelectric (PE) coupling to the TA and LA phonons is orders of magnitude lower. In the Bloch-Grüneisen (BG) regime, P ˜Te4(Te6) is predicted for unscreened (screened) el-ph interaction and P ˜n-1 /2(Pe˜n-3 /2) for both unscreened and screened el-ph interaction. The cooling power due to optical phonons is dominated by zero-order DP couplings and the Fröhlich interaction, and is found to be significantly reduced by the hot-phonon effect when the phonon relaxation time due to phonon-phonon scattering is large compared to the relaxation time due to el-ph scattering. The Te and n dependence of the hot-phonon distribution function is also studied. Our results for monolayer MoS2 are compared with those in conventional two-dimensional electron gases (2DEGs) as well as monolayer and bilayer graphene.

  11. Surfactant assisted control on optical, fluorescence and phonon lifetime in α-Bi2O3 microrods

    NASA Astrophysics Data System (ADS)

    Hariharan, S.; Udayabhaskar, R.; T. R., Ravindran; Karthikeyan, B.

    2016-06-01

    We report preparation of pure and surfactant added α-Bi2O3 microrods through simple chemical method at moderate temperature. Cetyltrimethyl ammonium bromide (CTAB) is used as a surfactant. X-ray diffraction (XRD), scanning electron microscopy (SEM), Fourier Transform Infrared (FTIR) spectroscopy, Raman spectroscopy, UV-Vis absorption and photoluminescence (PL) measurements were carried out to understand the effect of surfactant (CTAB) on structural, phonon and optical properties of the prepared material. It is observed that the crystallite size, optical band gap and the structural defects (oxygen vacancies) decreases due to the effect of surfactant. Raman spectral studies exhibit various phonon modes of Bi2O3 and also decrease in the FWHM of the phonon modes is observed after the addition of CTAB.

  12. A study of the structure and scattering mechanisms of subterahertz phonons in lithium fluoride single crystals and optical ceramics

    SciTech Connect

    Khazanov, E. N. Taranov, A. V.; Gainutdinov, R. V.; Akchurin, M. Sh.; Basiev, T. T.; Konyushkin, V. A.; Fedorov, P. P.; Kuznetsov, S. V.; Osiko, V. V.

    2010-06-15

    The methods of optical, electron, and atomic force microscopy (AFM) are applied to the study of the real structure of optical lithium fluoride ceramic obtained by hot deformation of single crystals. A comparative analysis is carried out of the scattering mechanisms of weakly nonequilibrium thermal phonons at liquid helium temperatures in LiF single crystals and ceramics. It is demonstrated that the phonon scattering in the original single crystals is determined by the forced vibrations of dislocations in the stress field of an elastic plane wave (a phonon), i.e., by the flutter mechanism. As the degree of deformation of the original material increases, the ceramics exhibit a change in the plastic deformation mechanisms, which leads to a decrease in the average size of grains and to an ordered structure. In this case, the dominant scattering is that by intergrain boundaries. The thickness and the acoustic impedance of these boundaries are evaluated.

  13. Off-axis phonon and photon propagation in porous silicon superlattices studied by Brillouin spectroscopy and optical reflectance

    SciTech Connect

    Parsons, L. C. Andrews, G. T.

    2014-07-21

    Brillouin light scattering experiments and optical reflectance measurements were performed on a pair of porous silicon-based optical Bragg mirrors which had constituent layer porosity ratios close to unity. For off-axis propagation, the phononic and photonic band structures of the samples were modeled as a series of intersecting linear dispersion curves. Zone-folding was observed for the longitudinal bulk acoustic phonon and the frequency of the probed zone-folded longitudinal phonon was shown to be dependent on the propagation direction as well as the folding order of the mode branch. There was no conclusive evidence of coupling between the transverse and the folded longitudinal modes. Two additional observed Brillouin peaks were attributed to the Rayleigh surface mode and a possible pseudo-surface mode. Both of these modes were dispersive, with the velocity increasing as the wavevector decreased.

  14. Surfactant assisted control on optical, fluorescence and phonon lifetime in α-Bi2O3 microrods.

    PubMed

    S, Hariharan; R, Udayabhaskar; T R, Ravindran; B, Karthikeyan

    2016-06-15

    We report preparation of pure and surfactant added α-Bi2O3 microrods through simple chemical method at moderate temperature. Cetyltrimethyl ammonium bromide (CTAB) is used as a surfactant. X-ray diffraction (XRD), scanning electron microscopy (SEM), Fourier Transform Infrared (FTIR) spectroscopy, Raman spectroscopy, UV-Vis absorption and photoluminescence (PL) measurements were carried out to understand the effect of surfactant (CTAB) on structural, phonon and optical properties of the prepared material. It is observed that the crystallite size, optical band gap and the structural defects (oxygen vacancies) decreases due to the effect of surfactant. Raman spectral studies exhibit various phonon modes of Bi2O3 and also decrease in the FWHM of the phonon modes is observed after the addition of CTAB. PMID:27031446

  15. Passive ring resonator micro-optical gyroscopes

    NASA Astrophysics Data System (ADS)

    Venediktov, V. Yu; Filatov, Yu V.; Shalymov, E. V.

    2016-05-01

    This paper reviews recent advances in passive micro-optical gyroscopes. In the last decade, most research effort in the area of micro-optical gyros has been concentrated on a configuration that takes advantage of a single-mode passive ring resonator, which is usually fabricated using integrated optical technologies. The dimensions of such micro-optical gyros are comparable to those of micromechanical gyroscopes (area of 10 to 100 mm2) and their sensitivity is considerably better than the sensitivity of the latter, approaching that of fibre-optic and laser gyros. Moreover, microoptical gyros can be made as a single integrated circuit, like the micromechanical gyros, but they have no movable parts, in contrast to their micromechanical counterparts. We also describe the development and investigation of micro-optical gyros produced in our studies.

  16. Correlated anomalous phase diffusion of coupled phononic modes in a sideband-driven resonator.

    PubMed

    Sun, F; Dong, X; Zou, J; Dykman, M I; Chan, H B

    2016-01-01

    The dynamical backaction from a periodically driven optical cavity can reduce the damping of a mechanical resonator, leading to parametric instability accompanied by self-sustained oscillations. Here we study experimentally and theoretically new aspects of the backaction and the discrete time-translation symmetry of a driven system using a micromechanical resonator with two nonlinearly coupled vibrational modes with strongly differing frequencies and decay rates. We find self-sustained oscillations in both the low- and high-frequency modes. Their frequencies and amplitudes are determined by the nonlinearity, which also leads to bistability and hysteresis. The phase fluctuations of the two modes show near-perfect anti-correlation, a consequence of the discrete time-translation symmetry. Concurrently, the phase of each mode undergoes anomalous diffusion. The phase variance follows a power law time dependence, with an exponent determined by the 1/f-type resonator frequency noise. Our findings enable compensating for the fluctuations using a feedback scheme to achieve stable frequency downconversion. PMID:27576597

  17. Protein Sensors Based on Optical Ring Resonators

    NASA Technical Reports Server (NTRS)

    Lin, Ying; Ksendzov, Alexander

    2006-01-01

    Prototype transducers based on integrated optical ring resonators have been demonstrated to be useful for detecting the protein avidin in extremely dilute solutions. In an experiment, one of the transducers proved to be capable of indicating the presence of avidin at a concentration of as little as 300 pM in a buffer solution a detection sensitivity comparable to that achievable by previously reported protein-detection techniques. These transducers are serving as models for the further development of integrated-optics sensors for detecting small quantities of other proteins and protein-like substances. The basic principle of these transducers was described in Chemical Sensors Based on Optical Ring Resonators (NPO-40601), NASA Tech Briefs, Vol. 29, No. 10 (October 2005), page 32. The differences between the present transducers and the ones described in the cited prior article lie in details of implementation of the basic principle. As before, the resonator in a transducer of the present type is a closed-circuit dielectric optical waveguide. The outermost layer of this waveguide, analogous to the optical cladding layer on an optical fiber, consists of a layer comprising sublayers having indices of refraction lower than that of the waveguide core. The outermost sublayer absorbs the chemical of interest (in this case, avidin). The index of refraction of the outermost sublayer changes with the concentration of absorbed avidin. The resonator is designed to operate with relatively strong evanescent-wave coupling between the outer sublayer and the electromagnetic field propagating along the waveguide core. By virtue of this coupling, the chemically induced change in the index of refraction of the outermost sublayer causes a measurable change in the spectrum of the resonator output.

  18. Lead-silicate glass optical microbubble resonator

    NASA Astrophysics Data System (ADS)

    Wang, Pengfei; Ward, Jonathan; Yang, Yong; Feng, Xian; Brambilla, Gilberto; Farrell, Gerald; Chormaic, Síle Nic

    2015-02-01

    Microbubble whispering gallery resonators have the potential to become key components in a variety of active and passive photonic circuit devices by offering a range of significant functionalities. Here, we report on the fabrication, optical characterization, and theoretical analysis of lead-silicate glass and optical microbubble resonators. Evanescent field coupling to the microbubbles was achieved using a 1 μm diameter, silica microfiber at a wavelength of circa 775 nm. High Q-factor modes were efficiently excited in both single-stem and two-stem, lead-silicate glass, and microbubble resonators, with bubble diameters of 38 μm (single-stem) and 48 μm (two-stem). Whispering gallery mode resonances with Q-factors as high as 2.3 × 105 (single-stem) and 7 × 106 (two-stem) were observed. By exploiting the high-nonlinearity of the lead-silicate glass, this work will act as a catalyst for studying a range of nonlinear optical effects in microbubbles, such as Raman scattering and four-wave mixing, at low optical powers.

  19. Lead-silicate glass optical microbubble resonator

    SciTech Connect

    Wang, Pengfei; Ward, Jonathan; Yang, Yong; Chormaic, Síle Nic; Feng, Xian; Brambilla, Gilberto; Farrell, Gerald

    2015-02-09

    Microbubble whispering gallery resonators have the potential to become key components in a variety of active and passive photonic circuit devices by offering a range of significant functionalities. Here, we report on the fabrication, optical characterization, and theoretical analysis of lead-silicate glass and optical microbubble resonators. Evanescent field coupling to the microbubbles was achieved using a 1 μm diameter, silica microfiber at a wavelength of circa 775 nm. High Q-factor modes were efficiently excited in both single-stem and two-stem, lead-silicate glass, and microbubble resonators, with bubble diameters of 38 μm (single-stem) and 48 μm (two-stem). Whispering gallery mode resonances with Q-factors as high as 2.3 × 10{sup 5} (single-stem) and 7 × 10{sup 6} (two-stem) were observed. By exploiting the high-nonlinearity of the lead-silicate glass, this work will act as a catalyst for studying a range of nonlinear optical effects in microbubbles, such as Raman scattering and four-wave mixing, at low optical powers.

  20. Effects of electron-optical phonon interactions on the polaron energy in a wurtzite ZnO/MgxZn1-xO quantum well

    NASA Astrophysics Data System (ADS)

    Zhao, Feng-Qi; Zhang, Min; Bai, Jin-Hua

    2015-09-01

    We investigated the properties of polarons in a wurtzite ZnO/MgxZn1-xO quantum well by adopting a modified Lee-Low-Pines variational method, giving the ground state energy, transition energy, and phonon contributions from various optical-phonon modes to the ground state energy as functions of the well width and Mg composition. In our calculations, we considered the effects of confined optical phonon modes, interface-optical phonon modes, and half-space phonon modes, as well as the anisotropy of the electron effective band mass, phonon frequency, and dielectric constant. Our numerical results indicate that the electron-optical phonon interactions importantly affect the polaronic energies in the ZnO/MgxZn1-xO quantum well. The electron-optical phonon interactions decrease the polaron energies. For quantum wells with narrower wells, the interface optical phonon and half-space phonon modes contribute more to the polaronic energies than the confined phonon modes. However, for wider quantum wells, the total contribution to the polaronic energy mainly comes from the confined modes. The contributions of the various phonon modes to the transition energy change differently with increasing well width. The contribution of the half-space phonons decreases slowly as the QW width increases, whereas the contributions of the confined and interface phonons reach a maximum at d ≈ 5.0 nm and then decrease slowly. However, the total contribution of phonon modes to the transition energy is negative and increases gradually with the QW width of d. As the composition x increases, the total contribution of phonons to the ground state energies increases slowly, but the total contributions of phonons to the transition energies decrease gradually. We analyze the physical reasons for these behaviors in detail. Project supported by the National Natural Science Foundation of China (Grant Nos. 11264027 and 11364030), the Project of Prairie Excellent Specialist of Inner Mongolia, China, and the

  1. Polar optical phonon states and their degenerative behaviors of wurtzite ZnO/MgZnO coupling quantum dots

    NASA Astrophysics Data System (ADS)

    Zhang, Li; Shi, J. J.

    2014-03-01

    Analytical polar optical phonon states in a wurtzite ZnO-based cylindrical coupling quantum dots (CQDs) with arbitrary number of quantum dots (QDs) are deduced and analyzed. It is found that there are four types of polar mixing optical phonon modes, i.e., the z-IO/ρ-QC modes, the z-PR/ρ-IO modes, the z-QC/ρ-QC modes and the z-HS/ρ-IO modes coexisting in the ZnO-based CQDs. Within the framework of the macroscopic dielectric continuum model, the dispersive equations are derived by using the transferring matrix method. And the Fröhlich electron-phonon interaction Hamiltonians are obtained via a standard procedure of field quantization. The relationships between the present ZnO-based CQDs and the ZnO-based quantum wells (QWs) or the nanowires (NWs) are analyzed, and the general features of phonon modes in ZnO-based low-dimensional quantum structures are concluded and discussed. Under certain conditions, the present theoretical results in wurtzite ZnO-based CQDs can be naturally degenerate into those in wurtzite ZnO-based single or double QDs, wurtzite NWs and QWs and even into cubic quantum confined structures. This just embodies the intrinsic consistency of phonon mode theories in low-dimensional confined systems with different confined dimensions. Due to the ternary mixing effect of MgxZn1-xO crystal, the dielectric functions of MgxZn1-xO crystals are quite complicated, and the phonon modes in ZnO-based quantum structures have both the features of phonon modes in anisotropic wurtzite confined systems and isotropic rock-salt crystal quantum systems. The characteristics of electron-phonon coupling strength in ZnO-based quantum systems are summarized. Very strong polaronic effect could be prognosticated and anticipated in ZnO-based low-dimensional quantum structures because of their quite large electron-phonon coupling constants. The theoretical results and conclusions described in this paper also can be looked on as a summary of phonon states and their general

  2. Invited Paper Optical Resonators For Associative Memory

    NASA Astrophysics Data System (ADS)

    Anderson, Dana Z.

    1986-06-01

    One can construct a memory having associative characteristics using optical resonators with an internal gain medium. The device operates on the principle that an optical resonator employing a holographic grating can have user prescribed eigenmodes. Information that is to be recalled is contained in the hologram. Each information entity (e.g. an image of a cat) defines an eigenmode of the resonator. The stored information is accessed by injecting partial information (e.g. an image of the cat's ear) into the resonator. The appropriate eigenmode is selected through a competitive process in a gain medium placed inside the resonator. With a net gain greater than one, the gain amplifies the field belonging to the eigenmode that most resembles the injected field; the other eigenmodes are suppressed via the competition for the gain. One can expect this device to display several intriguing features such as recall transitions and creativity. I will discuss some of the general properties of this class of devices and present the results from a series of experiments with a simple holographic resonator employing photorefractive gain.

  3. Slow Light in Coupled Resonator Optical Waveguides

    NASA Technical Reports Server (NTRS)

    Chang, Hongrok; Gates, Amanda L.; Fuller, Kirk A.; Gregory, Don A.; Witherow, William K.; Paley, Mark S.; Frazier, Donald O.; Smith, David D.; Curreri, Peter A. (Technical Monitor)

    2002-01-01

    Recently, we discovered that a splitting of the whispering gallery modes (WGMs) occurs in coupled resonator optical waveguides (CROWs), and that these split modes are of a higher Q than the single-resonator modes, leading to enormous circulating intensity magnification factors that dramatically reduce thresholds for nonlinear optical (NLO) processes. As a result of the enhancements in Q, pulses propagating at a split resonance can propagate much slower (faster) for over (under)-coupled structures, due to the modified dispersion near the split resonance. Moreover, when loss is considered, the mode-splitting may be thought of as analogous to the Autler-Townes splitting that occurs in atomic three-level lambda systems, i.e., it gives rise to induced transparency as a result of destructive interference. In under- or over-coupled CROWs, this coupled resonator induced transparency (CRIT) allows slow light to be achieved at the single-ring resonance with no absorption, while maintaining intensities such that NLO effects are maximized. The intensity magnification of the circulating fields and phase transfer characteristics are examined in detail.

  4. Magnetic plasmonic Fano resonance at optical frequency.

    PubMed

    Bao, Yanjun; Hu, Zhijian; Li, Ziwei; Zhu, Xing; Fang, Zheyu

    2015-05-13

    Plasmonic Fano resonances are typically understood and investigated assuming electrical mode hybridization. Here we demonstrate that a purely magnetic plasmon Fano resonance can be realized at optical frequency with Au split ring hexamer nanostructure excited by an azimuthally polarized incident light. Collective magnetic plasmon modes induced by the circular electric field within the hexamer and each of the split ring can be controlled and effectively hybridized by designing the size and orientation of each ring unit. With simulated results reproducing the experiment, our suggested configuration with narrow line-shape magnetic Fano resonance has significant potential applications in low-loss sensing and may serves as suitable elementary building blocks for optical metamaterials. PMID:25594885

  5. Temperature Sensors Based on WGM Optical Resonators

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy; Yu, Nan; Maleki, Lute; Itchenko, Vladimir; Matsko, Andrey; Strekalov, Dmitry

    2008-01-01

    A proposed technique for measuring temperature would exploit differences between the temperature dependences of the frequencies of two different electromagnetic modes of a whispering gallery-mode (WGM) optical resonator. An apparatus based on this technique was originally intended to be part of a control system for stabilizing a laser frequency in the face of temperature fluctuations. When suitably calibrated, apparatuses based on this technique could also serve as precise temperature sensors for purposes other than stabilization of lasers. A sensor according to the proposal would include (1) a transparent WGM dielectric resonator having at least two different sets of modes characterized by different thermo-optical constants and (2) optoelectronic instrumentation for measuring the difference between the temperature-dependent shifts of the resonance frequencies of the two sets of modes.

  6. Optical phonon frequencies in the quaternary CdTe1-x-ySexSy mixed system

    NASA Astrophysics Data System (ADS)

    Gupta, H. C.; Sood, Geeta; Malhotra, Jaishree; Tripathi, B. B.

    1986-08-01

    The optical phonon frequencies of the mixed-crystal system CdTe1-x-ySexSy are calculated theoretically by means of a concentration-dependent model utilizing the effect of nonrandomness. The calculations are in satisfactory agreement with the experimental results.

  7. Bioconjugation Strategies for Microtoroidal Optical Resonators

    PubMed Central

    Hunt, Heather K.; Soteropulos, Carol; Armani, Andrea M.

    2010-01-01

    The development of label-free biosensors with high sensitivity and specificity is of significant interest for medical diagnostics and environmental monitoring, where rapid and real-time detection of antigens, bacteria, viruses, etc., is necessary. Optical resonant devices, which have very high sensitivity resulting from their low optical loss, are uniquely suited to sensing applications. However, previous research efforts in this area have focused on the development of the sensor itself. While device sensitivity is an important feature of a sensor, specificity is an equally, if not more, important performance parameter. Therefore, it is crucial to develop a covalent surface functionalization process, which also maintains the device’s sensing capabilities or optical qualities. Here, we demonstrate a facile method to impart specificity to optical microcavities, without adversely impacting their optical performance. In this approach, we selectively functionalize the surface of the silica microtoroids with biotin, using amine-terminated silane coupling agents as linkers. The surface chemistry of these devices is demonstrated using X-ray photoelectron spectroscopy, and fluorescent and optical microscopy. The quality factors of the surface functionalized devices are also characterized to determine the impact of the chemistry methods on the device sensitivity. The resulting devices show uniform surface coverage, with no microstructural damage. This work represents one of the first examples of non-physisorption-based bioconjugation of microtoroidal optical resonators. PMID:22163409

  8. Coherence Phenomena in Coupled Optical Resonators

    NASA Technical Reports Server (NTRS)

    Smith, David D.

    2007-01-01

    Quantum coherence effects in atomic media such as electromagnetically-induced transparency and absorption, lasing without inversion, super-radiance and gain-assisted superluminality have become well-known in atomic physics. But these effects are not unique to atoms, nor are they uniquely quantum in nature, but rather are fundamental to systems of coherently coupled oscillators. In this talk I will review a variety of analogous photonic coherence phenomena that can occur in passive and active coupled optical resonators. Specifically, I will examine the evolution of the response that can occur upon the addition of a second resonator, to a single resonator that is side-coupled to a waveguide, as the coupling is increased, and discuss the conditions for slow and fast light propagation, coupled-resonator-induced transparency and absorption, lasing without gain, and gain-assisted superluminal pulse propagation. Finally, I will discuss the application of these systems to laser stabilization and gyroscopy.

  9. Optical Resonant Cavity in a Nanotaper

    SciTech Connect

    Lee, Sang Hyun; Goto, Takenari; Miyazaki, Hiroshi; Chang, Jiho; Yao, Takafumi

    2010-01-01

    The present study describes an optical resonant cavity in a nanotaper with scale reduction from micro to several nanometers. Both experimental results and a finite-difference time-domain (FDTD)-based simulation suggested that the nanometer-scale taper with a diameter similar to the wavelength of light acted as a mirror, which facilitated the formation of a laser cavity and caused lasing in ZnO nanotapers. As the light inside the nanotaper propagated toward the apex, the lateral mode was reduced and reflection occurred. This report suggests that use of the resonant optical cavities in nanotapers might result in novel active and passive optical components, which will broaden the horizons of photonic technology.

  10. Fourier-transform-based model for carrier transport in semiconductor heterostructures: Longitudinal optical phonon scattering

    NASA Astrophysics Data System (ADS)

    Lü, X.; Schrottke, L.; Grahn, H. T.

    2016-06-01

    We present scattering rates for electrons at longitudinal optical phonons within a model completely formulated in the Fourier domain. The total intersubband scattering rates are obtained by averaging over the intrasubband electron distributions. The rates consist of the Fourier components of the electron wave functions and a contribution depending only on the intersubband energies and the intrasubband carrier distributions. The energy-dependent part can be reproduced by a rational function, which allows for the separation of the scattering rates into a dipole-like contribution, an overlap-like contribution, and a contribution which can be neglected for low and intermediate carrier densities of the initial subband. For a balance between accuracy and computation time, the number of Fourier components can be adjusted. This approach facilitates an efficient design of complex heterostructures with realistic, temperature- and carrier density-dependent rates.

  11. Magnetic resonance imaging in Leber's optic neuropathy.

    PubMed Central

    Kermode, A G; Moseley, I F; Kendall, B E; Miller, D H; MacManus, D G; McDonald, W I

    1989-01-01

    Thirteen males with Leber's optic neuropathy had magnetic resonance imaging (MRI) of the brain, and in eight the optic nerves were imaged using STIR (Short Time Inversion Recovery) sequences. All optic nerve scans were abnormal. In seven with bilateral visual loss four showed bilateral increased optic nerve signal and three unilateral increase. The involvement was of the mid and posterior intra-orbital sections over three 5 mm slices or more with sparing of the anterior portion. One patient with unilateral visual loss had increased signal only on the affected side. Brain MRI was normal, in marked contrast to the findings in clinically isolated optic neuritis in which multiple white matter lesions are seen in the majority. Images PMID:2732742

  12. Magnetic resonance imaging of optic nerve

    PubMed Central

    Gala, Foram

    2015-01-01

    Optic nerves are the second pair of cranial nerves and are unique as they represent an extension of the central nervous system. Apart from clinical and ophthalmoscopic evaluation, imaging, especially magnetic resonance imaging (MRI), plays an important role in the complete evaluation of optic nerve and the entire visual pathway. In this pictorial essay, the authors describe segmental anatomy of the optic nerve and review the imaging findings of various conditions affecting the optic nerves. MRI allows excellent depiction of the intricate anatomy of optic nerves due to its excellent soft tissue contrast without exposure to ionizing radiation, better delineation of the entire visual pathway, and accurate evaluation of associated intracranial pathologies. PMID:26752822

  13. Doubly Resonant Optical Periodic Structure

    PubMed Central

    Alagappan, G.; Png, C. E.

    2016-01-01

    Periodic structures are well known in various branches of physics for their ability to provide a stopband. In this article, using optical periodic structures we showed that, when a second periodicity – very closed to the original periodicity is introduced, large number of states appears in the stopband corresponding to the first periodicity. In the limit where the two periods matches, we have a continuum of states, and the original stopband completely disappears. This intriguing phenomena is uncovered by noticing that, regardless of the proximities of the two periodicities, there is an array of spatial points where the dielectric functions corresponding to the two periodicities interfere destructively. These spatial points mimic photonic atoms by satisfying the standards equations of quantum harmonic oscillators, and exhibit lossless, atom-like dispersions. PMID:26853945

  14. Doubly Resonant Optical Periodic Structure.

    PubMed

    Alagappan, G; Png, C E

    2016-01-01

    Periodic structures are well known in various branches of physics for their ability to provide a stopband. In this article, using optical periodic structures we showed that, when a second periodicity - very closed to the original periodicity is introduced, large number of states appears in the stopband corresponding to the first periodicity. In the limit where the two periods matches, we have a continuum of states, and the original stopband completely disappears. This intriguing phenomena is uncovered by noticing that, regardless of the proximities of the two periodicities, there is an array of spatial points where the dielectric functions corresponding to the two periodicities interfere destructively. These spatial points mimic photonic atoms by satisfying the standards equations of quantum harmonic oscillators, and exhibit lossless, atom-like dispersions. PMID:26853945

  15. Wave-Chaotic Optical Resonators and Lasers

    NASA Astrophysics Data System (ADS)

    Stone, A. Douglas

    2001-10-01

    Deformed cylindrical and spherical dielectric optical resonators and lasers are analyzed from the perspective of non-linear dynamics and quantum chaos theory. In the short-wavelength limit such resonators behave like billiard systems with non-zero escape probability due to refraction. A ray model is introduced to predict the resonance lifetimes and emission patterns from such a cavity. A universal wavelength-independent broadening is predicted and found for large deformations of the cavity. However there are significant wave-chaotic corrections to the model which arise from chaos-assisted tunneling and dynamical localization effects. Highly directional emission from lasers based on these resonators is predicted from chaotic "whispering gallery" modes for index of refraction less than two. The detailed nature of the emission pattern can be understood from the nature of the phase-space flow in the billiard, and a dramatic variation of this pattern with index of refraction is found due to an effect we term "dynamical eclipsing". Semiconductor lasers of this type also show highly directional emission and high output power but from different modes associated with periodic orbits, both stable and unstable. A semiclassical approach to these modes is briefly reviewed. These asymmetric resonant cavities (ARCs) show promise as components in future integrated optical devices, providing perhaps the first application of quantum chaos theory.

  16. Infrared probe of spin-phonon coupling in antiferromagnetic honeycomb lattice compound Li2MnO3

    NASA Astrophysics Data System (ADS)

    Song, Seungjae; Lee, Sanghyun; Jeon, Seyoung; Park, Je-Geun; Moon, S. J.

    2015-12-01

    We investigated temperature-dependent infrared-active phonon modes of honeycomb Li2MnO3 which shows an antiferromagnetic transition at T N  =  36 K. In the far-infrared frequency region, we observed fourteen phonon modes. We obtained the temperature dependence of each phonon mode from the analysis of optical conductivity spectra by using the Lorentz and the Fano-type oscillator models. We found that the resonance frequencies of nine phonon modes showed an anomalous behavior near T N that should be attributed to the spin-phonon coupling. We calculated the magnitude of the spin-phonon coupling constant from the shift in the resonance frequencies of the phonon modes below T N. Our results suggest that Li2MnO3 is weakly frustrated and that spin-phonon coupling plays a role in antiferromagnetic ordering.

  17. Phonon-induced polariton superlattices.

    PubMed

    de Lima, M M; van der Poel, M; Santos, P V; Hvam, J M

    2006-07-28

    We show that the coherent interaction between microcavity polaritons and externally stimulated acoustic phonons forms a tunable polariton superlattice with a folded energy dispersion determined by the phonon population and wavelength. Under high phonon concentration, the strong confinement of the optical and excitonic polariton components in the phonon potential creates weakly coupled polariton wires with a virtually flat energy dispersion. PMID:16907587

  18. Resonance effects in thickness-dependent ultrafast carrier and phonon dynamics of topological insulator Bi2Se3.

    PubMed

    Kim, Sung; Shin, Dong Hee; Kim, Ju Hwan; Jang, Chan Wook; Park, Jun Woo; Lee, Hosun; Choi, Suk-Ho; Kim, Seung Hyun; Yee, Ki-Ju; Bansal, Namrata; Oh, Seongshik

    2016-01-29

    Resonance effects in the thickness-dependent ultrafast carrier and phonon dynamics of topological insulator Bi2Se3 are found irrespective of the kind of substrate by measuring thickness-dependent abrupt changes of pump-probe differential-reflectivity signals (ΔR/R) from Bi2Se3 thin films on four different substrates of poly- and single-crystalline (sc-) ZnO, sc-GaN and SiO2. The absolute peak intensity of the ΔR/R is maximized at ∼t C (6 ∼ 9 quintuple layers), which is not directly related to but is very close to the critical thickness below which the energy gap opens. The intensities of the two phonon modes deduced from the oscillatory behaviors superimposed on the ΔR/R profiles are also peaked at ∼t C for the four kinds of substrates, consistent with the thickness-dependent Raman-scattering behaviors. These resonant effects and others are discussed based on possible physical mechanisms including the effects of three-dimensional carrier depletion and intersurface coupling. PMID:26655693

  19. Resonance effects in thickness-dependent ultrafast carrier and phonon dynamics of topological insulator Bi2Se3

    NASA Astrophysics Data System (ADS)

    Kim, Sung; Shin, Dong Hee; Kim, Ju Hwan; Jang, Chan Wook; Park, Jun Woo; Lee, Hosun; Choi, Suk-Ho; Kim, Seung Hyun; Yee, Ki-Ju; Bansal, Namrata; Oh, Seongshik

    2016-01-01

    Resonance effects in the thickness-dependent ultrafast carrier and phonon dynamics of topological insulator Bi2Se3 are found irrespective of the kind of substrate by measuring thickness-dependent abrupt changes of pump-probe differential-reflectivity signals (ΔR/R) from Bi2Se3 thin films on four different substrates of poly- and single-crystalline (sc-) ZnO, sc-GaN and SiO2. The absolute peak intensity of the ΔR/R is maximized at ∼t C (6 ∼ 9 quintuple layers), which is not directly related to but is very close to the critical thickness below which the energy gap opens. The intensities of the two phonon modes deduced from the oscillatory behaviors superimposed on the ΔR/R profiles are also peaked at ∼t C for the four kinds of substrates, consistent with the thickness-dependent Raman-scattering behaviors. These resonant effects and others are discussed based on possible physical mechanisms including the effects of three-dimensional carrier depletion and intersurface coupling.

  20. Optical feshbach resonance using the intercombination transition.

    PubMed

    Enomoto, K; Kasa, K; Kitagawa, M; Takahashi, Y

    2008-11-14

    We report control of the scattering wave function by an optical Feshbach resonance effect using ytterbium atoms. The narrow intercombination line (1S0-3P1) is used for efficient control as proposed by Ciuryło et al. [Phys. Rev. A 71, 030701(R) (2005)10.1103/PhysRevA.71.030701]. The manipulation of the scattering wave function is monitored with the change of a photoassociation rate caused by another laser. The optical Feshbach resonance is especially efficient for isotopes with large negative scattering lengths such as 172Yb, and we have confirmed that the scattering phase shift divided by the wave number, which gives the scattering length in the zero energy limit, is changed by about 30 nm. PMID:19113335

  1. Optical spectral singularities as threshold resonances

    SciTech Connect

    Mostafazadeh, Ali

    2011-04-15

    Spectral singularities are among generic mathematical features of complex scattering potentials. Physically they correspond to scattering states that behave like zero-width resonances. For a simple optical system, we show that a spectral singularity appears whenever the gain coefficient coincides with its threshold value and other parameters of the system are selected properly. We explore a concrete realization of spectral singularities for a typical semiconductor gain medium and propose a method of constructing a tunable laser that operates at threshold gain.

  2. Laboratory investigation on the role of tubular shaped micro resonators phononic crystal insertion on the absorption coefficient of profiled sound absorber

    NASA Astrophysics Data System (ADS)

    Yahya, I.; Kusuma, J. I.; Harjana; Kristiani, R.; Hanina, R.

    2016-02-01

    This paper emphasizes the influence of tubular shaped microresonators phononic crystal insertion on the sound absorption coefficient of profiled sound absorber. A simple cubic and two different bodies centered cubic phononic crystal lattice model were analyzed in a laboratory test procedure. The experiment was conducted by using transfer function based two microphone impedance tube method refer to ASTM E-1050-98. The results show that sound absorption coefficient increase significantly at the mid and high-frequency band (600 - 700 Hz) and (1 - 1.6 kHz) when tubular shaped microresonator phononic crystal inserted into the tested sound absorber element. The increment phenomena related to multi-resonance effect that occurs when sound waves propagate through the phononic crystal lattice model that produce multiple reflections and scattering in mid and high-frequency band which increases the sound absorption coefficient accordingly

  3. The hydrogen-bond network of water supports propagating optical phonon-like modes

    DOE PAGESBeta

    Elton, Daniel C.; Fernández-Serra, Marivi

    2016-01-04

    The local structure of liquid water as a function of temperature is a source of intense research. This structure is intimately linked to the dynamics of water molecules, which can be measured using Raman and infrared spectroscopies. The assignment of spectral peaks depends on whether they are collective modes or single-molecule motions. Vibrational modes in liquids are usually considered to be associated to the motions of single molecules or small clusters. Using molecular dynamics simulations, here we find dispersive optical phonon-like modes in the librational and OH-stretching bands. We argue that on subpicosecond time scales these modes propagate through water’smore » hydrogen-bond network over distances of up to 2 nm. In the long wavelength limit these optical modes exhibit longitudinal–transverse splitting, indicating the presence of coherent long-range dipole–dipole interactions, as in ice. Lastly, our results indicate the dynamics of liquid water have more similarities to ice than previously thought.« less

  4. The hydrogen-bond network of water supports propagating optical phonon-like modes

    PubMed Central

    Elton, Daniel C.; Fernández-Serra, Marivi

    2016-01-01

    The local structure of liquid water as a function of temperature is a source of intense research. This structure is intimately linked to the dynamics of water molecules, which can be measured using Raman and infrared spectroscopies. The assignment of spectral peaks depends on whether they are collective modes or single-molecule motions. Vibrational modes in liquids are usually considered to be associated to the motions of single molecules or small clusters. Using molecular dynamics simulations, here we find dispersive optical phonon-like modes in the librational and OH-stretching bands. We argue that on subpicosecond time scales these modes propagate through water's hydrogen-bond network over distances of up to 2 nm. In the long wavelength limit these optical modes exhibit longitudinal–transverse splitting, indicating the presence of coherent long-range dipole–dipole interactions, as in ice. Our results indicate the dynamics of liquid water have more similarities to ice than previously thought. PMID:26725363

  5. The hydrogen bond network of water supports propagating optical phonon-like modes

    NASA Astrophysics Data System (ADS)

    Elton, Daniel; Fernadez-Serra, Marivi

    The local structure of liquid water as a function of temperature is a source of intense research. This structure is intimately linked to the dynamics of water molecules, which can be measured using Raman and infrared spectroscopies. Vibrational modes in liquids are usually considered to be associated to the motions of single molecules or small clusters. Previously, the librational Raman peaks of water were assigned to the librational motions of single molecules. By comparing experimental Raman and IR spectra we show these assignments are problematic. Using molecular dynamics simulations we study the k-dependent dielectric susceptibility of water. We find dispersive optical phonon-like modes in water's librational and OH stretching bands. We argue that on subpicosecond time scales these modes propagate through water's hydrogen bond network over distances of up to two nanometers. In the long wavelength limit these optical modes exhibit longitudinal-transverse splitting, indicating the presence of coherent long range dipole-dipole interactions. Studying how LO-TO splitting evolves with temperature may yield insight into how local structure changes. Our results indicate the dynamics of liquid water have more similarities to ice than previously thought. Reference: arXiv:1507.06363 This work was partially supported by DOE Award No. DE-FG02-09ER16052 (D.C.E.) and by DOE Early Career Award No. DE-SC0003871 (M.V.F.S.).

  6. Optical trapping apparatus, methods and applications using photonic crystal resonators

    SciTech Connect

    Erickson, David; Chen, Yih-Fan

    2015-06-16

    A plurality of photonic crystal resonator optical trapping apparatuses and a plurality optical trapping methods using the plurality of photonic crystal resonator optical trapping apparatuses include located and formed over a substrate a photonic waveguide that is coupled (i.e., either separately coupled or integrally coupled) with a photonic crystal resonator. In a particular embodiment, the photonic waveguide and the photonic crystal resonator comprise a monocrystalline silicon (or other) photonic material absent any chemical functionalization. In another particular embodiment, the photonic waveguide and the photonic crystal resonator comprise a silicon nitride material which when actuating the photonic crystal resonator optical trapping apparatus with a 1064 nanometer resonant photonic radiation wavelength (or other resonant photonic radiation wavelength in a range from about 700 to about 1200 nanometers) provides no appreciable heating of an aqueous sample fluid that is analyzed by the photonic crystal resonator optical trapping apparatus.

  7. Heavy-impurity resonance, hybridization, and phonon spectral functions in Fe1-xMxSi, M=Ir,Os

    SciTech Connect

    Delaire, O.; Al-Qasir, Iyad I.; May, Andrew F.; Sales, Brian C.; Niedziela, Jennifer L.; Ma, Jie; Matsuda, Masaaki; Abernathy, Douglas L.; Berlijn, Tom

    2015-03-31

    The vibrational behavior of heavy substitutional impurities (M=Ir,Os) in Fe1-xMxSi (x = 0, 0.02, 0.04, 0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. In this paper, our INS measurements on single-crystals mapped the four-dimensional dynamical structure factor, S(Q;E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers and increases electron-phonon coupling, leads to softened interatomic force-constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q,E) from INS through a Green's function model incorporating the phonon self-energy based on first-principles density functional theory (DFT) simulations. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Finally, our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity.

  8. Preface: Phonons 2007

    NASA Astrophysics Data System (ADS)

    Perrin, Bernard

    2007-06-01

    Conference logo The conference PHONONS 2007 was held 15-20 July 2007 in the Conservatoire National des Arts et Métiers (CNAM) Paris, France. CNAM is a college of higher technology for training students in the application of science to industry, founded by Henri Grégoire in 1794. This was the 12th International Conference on Phonon Scattering in Condensed Matter. This international conference series, held every 3 years, started in France at Sainte-Maxime in 1972. It was then followed by meetings at Nottingham (1975), Providence (1979), Stuttgart (1983), Urbana-Champaign (1986), Heidelberg (1989), Ithaca (1992), Sapporo (1995), Lancaster (1998), Dartmouth (2001) and St Petersburg (2004). PHONONS 2007 was attended by 346 delegates from 37 different countries as follows: France 120, Japan 45, Germany 25, USA 25, Russia 21, Italy 13, Poland 9, UK 9, Canada 7, The Netherlands 7, Finland 6, Spain 6, Taiwan 6, Greece 4, India 4, Israel 4, Ukraine 4, Serbia 3, South Africa 3, Argentina 2, Belgium 2, China 2, Iran 2, Korea 2, Romania 2, Switzerland 2, and one each from Belarus, Bosnia-Herzegovina, Brazil, Bulgaria, Egypt, Estonia, Mexico, Moldova, Morocco, Saudi Arabia, Turkey. There were 5 plenary lectures, 14 invited talks and 84 oral contributions; 225 posters were presented during three poster sessions. The first plenary lecture was given by H J Maris who presented fascinating movies featuring the motion of a single electron in liquid helium. Robert Blick gave us a review on the new possibilities afforded by nanotechnology to design nano-electomechanical systems (NEMS) and the way to use them to study elementary and fundamental processes. The growing interest for phonon transport studies in nanostructured materials was demonstrated by Arun Majumdar. Andrey Akimov described how ultrafast acoustic solitons can monitor the optical properties of quantum wells. Finally, Maurice Chapellier told us how

  9. Miniature fiber optic surface plasmon resonance biosensors

    NASA Astrophysics Data System (ADS)

    Slavik, Radan; Brynda, Eduard; Homola, Jiri; Ctyroky, Jiri

    1999-01-01

    A novel design of surface plasmon resonance fiber optic sensor is reported which leads to a compact, highly miniaturized sensing element with excellent sensitivity. The sensing device is based on a side-polished single-mode optical fiber with a thin metal overlayer supporting surface plasmon waves. The strength of interaction between a fiber mode and a surface plasmon wave depends strongly on the refractive index near the sensing surface. Therefore, refractive index changes associated with biospecific interaction between antibodies immobilized on the sensor and antigen molecules can be monitored by measuring light intensity variations. Detection of horse radish peroxidase (HRP) of the concentration of 100 ng/ml has been accomplished using the fiber optic sensor with a matrix of monoclonal antibodies against HRP immobilized on the sensor surface.

  10. Fermi resonance in the phonon spectra of quaternary chalcogenides of the type Cu2ZnGeS4.

    PubMed

    Valakh, M Ya; Litvinchuk, A P; Dzhagan, V M; Yukhymchuk, V O; Yaremko, A M; Romanyuk, Yu A; Guc, M; Bodnar, I V; Pérez-Rodríguez, A; Zahn, D R T

    2016-02-17

    The experimental resonant and non-resonant Raman scattering spectra of the kesterite structural modification of Cu2ZnGeS4 single crystals are reported. The results are compared with those calculated theoretically within the density functional perturbation theory. For the majority of lines a good agreement (within 2-5 cm(-1)) is established between experimental and calculated mode frequencies. However, several dominant spectral lines, in particular the two intense fully symmetric modes, are found to deviate from the calculated values by as much as 20 cm(-1). A possible reason for this discrepancy is found to be associated with the Fermi resonant interaction between one and two-phonon vibrational excitations. The modelling of spectra, which takes into account the symmetry of interacting states, allows a qualitative description of the observed experimental findings. Due to the similarity of the vibrational spectra of Cu2A (II) B (IV) S4 (A  =  Zn, Mn, Cd; B  =  Sn, Ge, Si) chalcogenides, Fermi resonance is argued to be a general phenomenon for this class of compounds. PMID:26795711

  11. Fermi resonance in the phonon spectra of quaternary chalcogenides of the type Cu2ZnGeS4

    NASA Astrophysics Data System (ADS)

    Valakh, M. Ya; Litvinchuk, A. P.; Dzhagan, V. M.; Yukhymchuk, V. O.; Yaremko, A. M.; Romanyuk, Yu A.; Guc, M.; Bodnar, I. V.; Pérez-Rodríguez, A.; Zahn, D. R. T.

    2016-02-01

    The experimental resonant and non-resonant Raman scattering spectra of the kesterite structural modification of Cu2ZnGeS4 single crystals are reported. The results are compared with those calculated theoretically within the density functional perturbation theory. For the majority of lines a good agreement (within 2-5 cm-1) is established between experimental and calculated mode frequencies. However, several dominant spectral lines, in particular the two intense fully symmetric modes, are found to deviate from the calculated values by as much as 20 cm-1. A possible reason for this discrepancy is found to be associated with the Fermi resonant interaction between one and two-phonon vibrational excitations. The modelling of spectra, which takes into account the symmetry of interacting states, allows a qualitative description of the observed experimental findings. Due to the similarity of the vibrational spectra of Cu2A II B IV S4 (A  =  Zn, Mn, Cd; B  =  Sn, Ge, Si) chalcogenides, Fermi resonance is argued to be a general phenomenon for this class of compounds.

  12. Strong Optical-Mechanical Coupling in a Vertical GaAs/AlAs Microcavity for Subterahertz Phonons and Near-Infrared Light

    NASA Astrophysics Data System (ADS)

    Fainstein, A.; Lanzillotti-Kimura, N. D.; Jusserand, B.; Perrin, B.

    2013-01-01

    We show that distributed Bragg reflector GaAs/AlAs vertical cavities designed to confine photons are automatically optimal to confine phonons of the same wavelength, strongly enhancing their interaction. We study the impulsive generation of intense coherent and monochromatic acoustic phonons by following the time evolution of the elastic strain in picosecond-laser experiments. Efficient optical detection is assured by the strong phonon backaction on the high-Q optical cavity mode. Large optomechanical factors are reported (˜THz/nm range). Pillar cavities based in these structures are predicted to display picogram effective masses, almost perfect sound extraction, and threshold powers for the stimulated emission of phonons in the range μW-mW, opening the way for the demonstration of phonon “lasing” by parametric instability in these devices.

  13. Tuning characteristic of band gap and waveguide in a multi-stub locally resonant phononic crystal plate

    NASA Astrophysics Data System (ADS)

    Wang, Xiao-Peng; Jiang, Ping; Chen, Tian-Ning; Zhu, Jian

    2015-10-01

    In this paper, the tuning characteristics of band gaps and waveguides in a locally resonant phononic crystal structure, consisting of multiple square stubs deposited on a thin homogeneous plate, are investigated. Using the finite element method and supercell technique, the dispersion relationships and power transmission spectra of those structures are calculated. In contrast to a system of one square stub, systems of multiple square stubs show wide band gaps at lower frequencies and an increased quantity of band gaps at higher frequencies. The vibration modes of the band gap edges are analyzed to clarify the mechanism of the generation of the lowest band gap. Additionally, the influence of the stubs arrangement on the band gaps in multi-stub systems is investigated. The arrangements of the stubs were found to influence the band gaps; this is critical to understand for practical applications. Based on this finding, a novel method to form defect scatterers by changing the arrangement of square stubs in a multi-stub perfect phononic crystal plate was developed. Defect bands can be induced by creating defects inside the original complete band gaps. The frequency can then be tuned by changing the defect scatterers' stub arrangement. These results will help in fabricating devices such as acoustic filters and waveguides whose band frequency can be modulated.

  14. Phonon Lifetime Measurement by Stimulated Brillouin Scattering Slow Light Technique in Optical Fiber

    NASA Astrophysics Data System (ADS)

    Chen, Wei; Meng, Zhou; Zhou, Hui-Juan

    2013-07-01

    Phonon lifetime is a significant parameter in the process of stimulated Brillouin scattering (SBS). In the present study, SBS slow light technique is used to measure phonon lifetime. Brillouin bandwidth is divided into natural, spontaneous and stimulated bandwidth. Compared with the traditional heterodyne-detection and pump-probe techniques, the natural Brillouin bandwidth can be obtained by SBS slow light technique, which equals the reciprocal of phonon lifetime and has no relations with the pump power. Another advantage of this technique is that the effect of polarization can be excluded. The natural Brillouin bandwidth is measured to be ~50 MHz and the phonon lifetime ~3.2 ns in the conventional single-mode fiber (SMF) at room temperature and zero strain. The obtained results are guidable in applications where the phonon lifetime information is a requisite such as phase conjugation and pulse compression.

  15. Silicon single-crystal cryogenic optical resonator.

    PubMed

    Wiens, Eugen; Chen, Qun-Feng; Ernsting, Ingo; Luckmann, Heiko; Rosowski, Ulrich; Nevsky, Alexander; Schiller, Stephan

    2014-06-01

    We report on the demonstration and characterization of a silicon optical resonator for laser frequency stabilization, operating in the deep cryogenic regime at temperatures as low as 1.5 K. Robust operation was achieved, with absolute frequency drift less than 20 Hz over 1 h. This stability allowed sensitive measurements of the resonator thermal expansion coefficient (α). We found that α=4.6×10(-13)  K(-1) at 1.6 K. At 16.8 K α vanishes, with a derivative equal to -6×10(-10)  K(-2). The temperature of the resonator was stabilized to a level below 10 μK for averaging times longer than 20 s. The sensitivity of the resonator frequency to a variation of the laser power was also studied. The corresponding sensitivities and the expected Brownian noise indicate that this system should enable frequency stabilization of lasers at the low-10(-17) level. PMID:24876023

  16. Simultaneous occurrence of structure-directed and particle-resonance-induced phononic gaps in colloidal films.

    PubMed

    Still, T; Cheng, W; Retsch, M; Sainidou, R; Wang, J; Jonas, U; Stefanou, N; Fytas, G

    2008-05-16

    We report on the observation of two hypersonic phononic gaps of different nature in three-dimensional colloidal films of nanospheres using Brillouin light scattering. One is a Bragg gap occurring at the edge of the first Brillouin zone along a high-symmetry crystal direction. The other is a hybridization gap in crystalline and amorphous films, originating from the interaction of the band of quadrupole particle eigenmodes with the acoustic effective-medium band, and its frequency position compares well with the computed lowest eigenfrequency. Structural disorder eliminates the Bragg gap, while the hybridization gap is robust. PMID:18518452

  17. Resonant phase jump with enhanced electric field caused by surface phonon polariton in terahertz region.

    PubMed

    Okada, Takanori; Nagai, Masaya; Tanaka, Koichiro

    2008-04-14

    We investigated surface phonon polariton in cesium iodide with terahertz time-domain attenuated total reflection method in Otto configuration, which gives us both information on amplitude and phase of surface electromagnetic mode directly. Systematic experiments with precise control of the distance between a prism and an active material show that the abrupt change of pi-phase jump appears sensitively under polariton picture satisfied when the local electric field at the interface becomes a maximum. This demonstration will open the novel phase-detection terahertz sensor using the active medium causing the strong enhancement of terahertz electric field. PMID:18542668

  18. A self-stabilized coherent phonon source driven by optical forces

    PubMed Central

    Navarro-Urrios, D.; Capuj, N. E.; Gomis-Bresco, J.; Alzina, F.; Pitanti, A.; Griol, A.; Martínez, A.; Sotomayor Torres, C. M.

    2015-01-01

    We report a novel injection scheme that allows for “phonon lasing” in a one-dimensional opto-mechanical photonic crystal, in a sideband unresolved regime and with cooperativity values as low as 10−2. It extracts energy from a cw infrared laser source and is based on the triggering of a thermo-optical/free-carrier-dispersion self-pulsing limit-cycle, which anharmonically modulates the radiation pressure force. The large amplitude of the coherent mechanical motion acts as a feedback that stabilizes and entrains the self-pulsing oscillations to simple fractions of the mechanical frequency. A manifold of frequency-entrained regions with two different mechanical modes (at 54 and 122 MHz) are observed as a result of the wide tuneability of the natural frequency of the self-pulsing. The system operates at ambient conditions of pressure and temperature in a silicon platform, which enables its exploitation in sensing, intra-chip metrology or time-keeping applications. PMID:26503448

  19. All optical modulator based on silicon resonator

    NASA Astrophysics Data System (ADS)

    Pinhas, Hadar; Bidani, Liron; Baharav, Oded; Sinvani, Moshe; Danino, Meir; Zalevsky, Zeev

    2015-08-01

    In this paper we present an all-optical silicon modulator, where a silicon slab (450 μm) thick is coated on both sides to get a Fabry-Perot resonator for laser beam at wavelength of 1550nm. Most of the modulators discussed in literature, are driven by electrical field rather than by light. We investigate new approaches regarding the dependence of the absorption of the optical signal on the control laser pulse at 532 nm having 5nm pulse width. Our silicon based Fabry-Perot resonator increases the intrinsic c-Si finesse to >10, instead of the uncoated silicon with natural finesse of 2.5. The improved finesse is shown to have significant effect on the modulation depth using a pulsed laser. A modulation of 12dB was attained. The modulation is ascribed to two different effects - The Plasma Dispersion Effect (PDE) and the Thermo- Optic Effect (TOE). The PDE causes increase in the signal absorption in silicon via the absorption of the control laser light. On top of that, the transmission of the signal can decrease dramatically in high finesse resonators due to change in the refractive index due to TOE. The changes in the signal's absorption coefficient and in the refractive index are the result of incremental change in the concentration of free carriers. The TOE gives rise to higher refractive index as opposed to the PDE which triggers a decrease in the refractive index. Finally, tradeoff considerations are presented on how to modify one effect to counter the other one, leading to an optimal device having reduced temperature dependence.

  20. Symmetry-adapted tight-binding calculations of the totally symmetric A1 phonons of single-walled carbon nanotubes and their resonant Raman intensity

    NASA Astrophysics Data System (ADS)

    Popov, Valentin N.; Lambin, Philippe

    2007-03-01

    The atomistic calculations of the physical properties of perfect single-walled carbon nanotubes based on the use of the translational symmetry of the nanotubes face increasing computational difficulties for most of the presently synthesized nanotubes with up to a few thousand atoms in the unit cell. This difficulty can be circumvented by use of the helical symmetry of the nanotubes and a two-atom unit cell. We present the results of such symmetry-adapted tight-binding calculations of the totally symmetric A1 phonons (the RBM and the G-band modes) and their resonant Raman intensity for several hundred nanotubes. In particular, we show that (1) the frequencies and the resonant Raman intensity of the RBM and the G-band modes show diameter and chirality dependence and family patterns, (2) the strong electron- A1LO phonon interactions in metallic nanotubes lead to Kohn anomalies at the zone center, (3) the G-band consists of a subband due to A1LO phonons of semiconducting tubes centered at ∼1593 cm -1, a subband of A1TO phonons at ∼1570 cm -1, and a subband of A1LO phonons of metallic tubes at ∼1540 cm -1. The latter prediction confirms previous theoretical results but disagrees with the commonly adopted assignment of the G-band features.

  1. Optical filter having coupled whispering-gallery-mode resonators

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy (Inventor); Ilchenko, Vladimir (Inventor); Maleki, Lutfollah (Inventor); Handley, Timothy A. (Inventor)

    2006-01-01

    Optical filters having at least two coupled whispering-gallery-mode (WGM) optical resonators to produce a second order or higher order filter function with a desired spectral profile. At least one of the coupled WGM optical resonators may be tunable by a control signal to adjust the filtering function.

  2. Propagating optical-phonon modes and their electron-phonon interactions in wurtzite GaN/AlxGa1-xN quantum wells

    NASA Astrophysics Data System (ADS)

    Shi, Jun-Jie; Chu, Xing-Li; Goldys, E. M.

    2004-09-01

    The equation of motion for the p -polarization field in an arbitrary wurtzite multilayer heterostructure is solved for the propagating optical-phonon (POP) modes in the framework of the dielectric-continuum model and Loudon’s uniaxial crystal model. The polarization eigenvector, the dispersion relation, and the electron-propagating-phonon (EPP) interaction Fröhlich-like Hamiltonian are derived. The analytical formulas can be directly applied to single heterojunctions, single and multiple quantum wells (QW’s), and superlattices. The dispersion relations of the POP modes and the EPP coupling functions are investigated for a given GaN/Al0.15Ga0.85N single QW with full account of the strains of QW structures and the anisotropy effects of wurtzite crystals. We find that there are infinite POP branches, which can be denoted by a quantum number n(n=1,2,…) , with definite symmetry with respect to the center of symmetry of the QW structure. The dispersion of the POP modes with smaller n is more obvious than for larger n . Moreover, the modes with smaller n are much more important for the EPP interactions than the modes with larger n . In most cases, it is enough to consider the modes with n=1,2,…,10 for the EPP interactions in a single QW. The long-wavelength POP modes are much more important for the EPP interactions. Furthermore, the strain effects of the QW structures have a strong influence on the dispersion of the POP modes. The strength of the EPP interactions is markedly increased due to the strains of the QW structures.

  3. PHONONS IN INTRINSIC JOSEPHSON SYSTEMS

    SciTech Connect

    C. PREIS; K. SCHMALZL; ET AL

    2000-10-01

    Subgap structures in the I-V curves of layered superconductors are explained by the excitation of phonons by Josephson oscillations. In the presence of a magnetic field applied parallel to the layers additional structures due to fluxon motion appear. Their coupling with phonons is investigated theoretically and a shift of the phonon resonances in strong magnetic fields is predicted.

  4. Nonlinear optics and crystalline whispering gallery mode resonators

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey B.; Savchenkov, Anatoliy A.; Ilchenko, Vladimir S.; Maleki, Lute

    2004-01-01

    We report on our recent results concerning fabrication of high-Q whispering gallery mode (WGM) crystalline resonators, and discuss some possible applications of lithium niobate WGM resonators in nonlinear optics and photonics. In particular, we demonstrate experimentally a tunable third-order optical filter fabricated from the three metalized resonators; and report observation of parametric frequency dobuling in a WGM resonator made of periodically poled lithium niobate (PPLN).

  5. Electron-Phonon Coupling in the Bulk of Anatase TiO2 Measured by Resonant Inelastic X-Ray Spectroscopy.

    PubMed

    Moser, S; Fatale, S; Krüger, P; Berger, H; Bugnon, P; Magrez, A; Niwa, H; Miyawaki, J; Harada, Y; Grioni, M

    2015-08-28

    We investigate the polaronic ground state of anatase TiO2 by bulk-sensitive resonant inelastic x-ray spectroscopy (RIXS) at the Ti L3 edge. We find that the formation of the polaron cloud involves a single 95 meV phonon along the c axis, in addition to the 108 meV ab-plane mode previously identified by photoemission. The coupling strength to both modes is the same within error bars, and it is unaffected by the carrier density. These data establish RIXS as a directional bulk-sensitive probe of electron-phonon coupling in solids. PMID:26371668

  6. Measurement of optical Feshbach resonances in an ideal gas.

    PubMed

    Blatt, S; Nicholson, T L; Bloom, B J; Williams, J R; Thomsen, J W; Julienne, P S; Ye, J

    2011-08-12

    Using a narrow intercombination line in alkaline earth atoms to mitigate large inelastic losses, we explore the optical Feshbach resonance effect in an ultracold gas of bosonic (88)Sr. A systematic measurement of three resonances allows precise determinations of the optical Feshbach resonance strength and scaling law, in agreement with coupled-channel theory. Resonant enhancement of the complex scattering length leads to thermalization mediated by elastic and inelastic collisions in an otherwise ideal gas. Optical Feshbach resonance could be used to control atomic interactions with high spatial and temporal resolution. PMID:21902391

  7. Plasmonic modification of electron-longitudinal-optical phonon coupling in Ag-nanoparticle embedded InGaN/GaN quantum wells

    NASA Astrophysics Data System (ADS)

    Llopis, Antonio; Pereira, Sérgio M. S.; Watson, Ian M.; Neogi, Arup

    2014-09-01

    Surface plasmon enhanced GaN and InGaN quantum wells (QWs) show promise for use as room-temperature light emitters. The effectiveness of the plasmon enhancement, however, is limited by the strong electron/hole and longitudinal optical phonon coupling found in the III-V nitrides. The electron-phonon coupling within semiconductor QWs has been modified using silver nanoparticles embedded within the QWs. Direct evidence is provided for this change via confocal Raman spectroscopy of the samples. This evidence is augmented by Angle-dependent photoluminescence experiments which show the alteration of the electron-phonon coupling strength through measurement of the emitted phonon replicas. Together these demonstrate a direct modification of carrier-phonon interactions within the system, opening up the possibility of controlling the coupling strength to produce high-efficiency room-temperature light emitters.

  8. Heavy ion Coulomb excitation and gamma decay studies of the one and two phonon giant dipole resonances in {sup 208}Pb and {sup 209}Bi

    SciTech Connect

    Mueller, P.E.; Beene, J.R.; Bertrand, F.E.

    1993-12-01

    Projectile -- photon coincidences were measured for the scattering of an 80 MeV/nucleon {sup 64}Zn beam from {sup 208}Pb and {sup 209}Bi targets at the GANIL heavy ion accelerator facility. Projectile-like particles between 0.5{degrees} and 4.5{degrees} relative to the incident beam direction were detected in the SPEG energy loss spectrometer where their momentum, charge, and mass were determined. Photons were detected in the BaF{sub 2} scintillation detector array TAPS. Light charged particles produced in the reaction were detected in the KVI Forward Wall. The analysis of the data acquired in this experiment is focused on three different phenomena: (1) the two phonon giant dipole resonance, (2) time dependence of the decay of the one phonon giant dipole resonance, and (3) giant resonance strength in projectile nuclei.

  9. Magneto-optical properties of trions in non-blinking charged nanocrystals reveal an acoustic phonon bottleneck.

    PubMed

    Fernée, Mark J; Sinito, Chiara; Louyer, Yann; Potzner, Christian; Nguyen, Tich-Lam; Mulvaney, Paul; Tamarat, Philippe; Lounis, Brahim

    2012-01-01

    Charged quantum dots provide an important platform for a range of emerging quantum technologies. Colloidal quantum dots in particular offer unique advantages for such applications (facile synthesis, manipulation and compatibility with a wide range of environments), especially if stable charged states can be harnessed in these materials. Here we engineer the CdSe nanocrystal core and shell structure to efficiently ionize at cryogenic temperatures, resulting in trion emission with a single sharp zero-phonon line and a mono exponential decay. Magneto-optical spectroscopy enables direct determination of electron and hole g-factors. Spin relaxation is observed in high fields, enabling unambiguous identification of the trion charge. Importantly, we show that spin flips are completely inhibited for Zeeman splittings below the low-energy bound for confined acoustic phonons. This reveals a characteristic unique to colloidal quantum dots that will promote the use of these versatile materials in challenging quantum technological applications. PMID:23250417

  10. Magneto-optical properties of trions in non-blinking charged nanocrystals reveal an acoustic phonon bottleneck

    NASA Astrophysics Data System (ADS)

    Fernée, Mark J.; Sinito, Chiara; Louyer, Yann; Potzner, Christian; Nguyen, Tich-Lam; Mulvaney, Paul; Tamarat, Philippe; Lounis, Brahim

    2012-12-01

    Charged quantum dots provide an important platform for a range of emerging quantum technologies. Colloidal quantum dots in particular offer unique advantages for such applications (facile synthesis, manipulation and compatibility with a wide range of environments), especially if stable charged states can be harnessed in these materials. Here we engineer the CdSe nanocrystal core and shell structure to efficiently ionize at cryogenic temperatures, resulting in trion emission with a single sharp zero-phonon line and a mono exponential decay. Magneto-optical spectroscopy enables direct determination of electron and hole g-factors. Spin relaxation is observed in high fields, enabling unambiguous identification of the trion charge. Importantly, we show that spin flips are completely inhibited for Zeeman splittings below the low-energy bound for confined acoustic phonons. This reveals a characteristic unique to colloidal quantum dots that will promote the use of these versatile materials in challenging quantum technological applications.

  11. Fiber-optic integration and efficient detection schemes for optomechanical resonators

    NASA Astrophysics Data System (ADS)

    Cohen, Justin D.

    optomechanical resonators to optical fibers, with an emphasis on fabrication processes and optical characterization. I will then proceed to describe a few experiments enabled by the fiber couplers. The first studies the performance of an optomechanical resonator as a precise sensor for continuous position measurement. The sensitivity of the measurement, limited by the detection efficiency of intracavity photons, is compared to the standard quantum limit imposed by the quantum properties of the laser probe light. The added noise of the measurement is seen to fall within a factor of 3 of the standard quantum limit, representing an order of magnitude improvement over previous experiments utilizing optomechanical crystals, and matching the performance of similar measurements in the microwave domain. The next experiment uses single photon counting to detect individual phonon emission and absorption events within the nanomechanical oscillator. The scattering of laser light from mechanical motion produces correlated photon-phonon pairs, and detection of the emitted photon corresponds to an effective phonon counting scheme. In the process of scattering, the coherence properties of the mechanical oscillation are mapped onto the reflected light. Intensity interferometry of the reflected light then allows measurement of the temporal coherence of the acoustic field. These correlations are measured for a range of experimental conditions, including the optomechanical amplification of the mechanics to a self-oscillation regime, and comparisons are drawn to a laser system for phonons. Finally, prospects for using phonon counting and intensity interferometry to produce non-classical mechanical states are detailed following recent proposals in literature.

  12. Parametric resonance-induced time-convolutionless master equation breakdown in finite size exciton-phonon systems.

    PubMed

    Pouthier, Vincent

    2010-09-29

    A detailed analysis is performed to show that the second order time-convolutionless master equation fails to describe the exciton-phonon dynamics in a finite size lattice. To proceed, special attention is paid to characterizing the coherences of the exciton reduced density matrix. These specific elements measure the ability of the exciton to develop superimpositions involving the vacuum and the one-exciton states. It is shown that the coherences behave as wavefunctions whose dynamics is governed by a time-dependent effective Hamiltonian defined in terms of the so-called time-dependent relaxation operator. Due to the confinement, quantum recurrences provide to the relaxation operator an almost periodic nature, so the master equation reduces to a linear system of differential equations with almost periodic coefficients. We show that, in accordance with the Floquet theory, unstable solutions emerge due to parametric resonances involving specific frequencies of the relaxation operator and specific excitonic eigenfrequencies. These resonances give rise to an unphysical exponential growth of the coherences, indicating the breakdown of the second order master equation. PMID:21386551

  13. Scanning Tunneling Optical Resonance Microscopy Developed

    NASA Technical Reports Server (NTRS)

    Bailey, Sheila G.; Raffaelle, Ryne P.; Lau, Janis E.; Jenkins, Phillip P.; Castro, Stephanie L.; Tin, Padetha; Wilt, David M.; Pal, Anna Maria; Fahey, Stephen D.

    2004-01-01

    The ability to determine the in situ optoelectronic properties of semiconductor materials has become especially important as the size of device architectures has decreased and the development of complex microsystems has increased. Scanning Tunneling Optical Resonance Microscopy, or STORM, can interrogate the optical bandgap as a function of its position within a semiconductor micro-structure. This technique uses a tunable solidstate titanium-sapphire laser whose output is "chopped" using a spatial light modulator and is coupled by a fiber-optic connector to a scanning tunneling microscope in order to illuminate the tip-sample junction. The photoenhanced portion of the tunneling current is spectroscopically measured using a lock-in technique. The capabilities of this technique were verified using semiconductor microstructure calibration standards that were grown by organometallic vapor-phase epitaxy. Bandgaps characterized by STORM measurements were found to be in good agreement with the bulk values determined by transmission spectroscopy and photoluminescence and with the theoretical values that were based on x-ray diffraction results.

  14. Optical cavity resonator in an expanding universe

    NASA Astrophysics Data System (ADS)

    Kopeikin, Sergei M.

    2015-02-01

    We study the cosmological evolution of frequency of a standing electromagnetic wave in a resonant optical cavity placed to the expanding manifold described by the Robertson-Walker metric. Because of the Einstein principle of equivalence (EEP), one can find a local coordinate system (a local freely falling frame), in which spacetime is locally Minkowskian. However, due to the conformal nature of the Robertson-Walker metric the conventional transformation to the local inertial coordinates introduces ambiguity in the physical interpretation of the local time coordinate, . Therefore, contrary to a common-sense expectation, a straightforward implementation of EEP alone does not allow us to unambiguously decide whether atomic clocks based on quantum transitions of atoms, ticks at the same rate as the clocks based on electromagnetic modes of a cavity. To resolve this ambiguity we have to analyse the cavity rigidity and the oscillation of its electromagnetic modes in an expanding universe by employing the full machinery of the Maxwell equations irrespectively of the underlying theory of gravity. We proceed in this way and found out that the size of the cavity and the electromagnetic frequency experience an adiabatic drift in conformal (unphysical) coordinates as the universe expands in accordance with the Hubble law. We set up the oscillation equation for the resonant electromagnetic modes, solve it by the WKB approximation, and reduce the coordinate-dependent quantities to their counterparts measured by a local observer who counts time with atomic clock. The solution shows that there is a perfect mutual cancellation of the adiabatic drift of cavity's frequency by space transformation to local coordinates and the time counted by the clocks based on electromagnetic modes of cavity has the same rate as that of atomic clocks. We conclude that if general relativity is correct and the local expansion of space is isotropic there should be no cosmological drift of frequency of a

  15. Coherent acoustic phonon oscillation accompanied with backward acoustic pulse below exciton resonance in a ZnO epifilm on oxide-buffered Si(1 1 1)

    NASA Astrophysics Data System (ADS)

    Lin, Ja-Hon; Shen, Yu-Kai; Liu, Wei-Rein; Lu, Chia-Hui; Chen, Yao-Hui; Chang, Chun-peng; Lee, Wei-Chin; Hong, Minghwei; Kwo, Jueinai-Raynien; Hsu, Chia-Hung; Hsieh, Wen-Feng

    2016-08-01

    Unlike coherent acoustic phonons (CAPs) generated from heat induced thermal stress by the coated Au film, we demonstrated the oscillation from c-ZnO epitaxial film on oxide buffered Si through a degenerate pump–probe technique. As the excited photon energy was set below the exciton resonance, the electronic stress that resulted from defect resonance was used to induce acoustic wave. The damped oscillation revealed a superposition of a high frequency and long decay CAP signal with a backward propagating acoustic pulse which was generated by the absorption of the penetrated pump beam at the Si surface and selected by the ZnO layer as the acoustic resonator.

  16. Calomel-made crystalline acousto-optical cell designed for an advanced regime of noncollinear two-phonon light scattering

    NASA Astrophysics Data System (ADS)

    Shcherbakov, Alexandre S.; Arellanes, Adan Omar

    2016-03-01

    We study the potentials of a wide-aperture crystalline calomel-made acousto-optical cell. Characterizing this cell is nontrivial due to the chosen regime based on an advanced noncollinear two-phonon light scattering. Recently revealed important features of this phenomenon are essentially exploited in the cell and are investigated in more detail. These features can be observed more easily and simply in tetragonal crystals, e.g., calomel, exhibiting specific acousto-optical nonlinearity caused by the acoustic waves of finite amplitude. This parametric nonlinearity manifests itself at low acoustic powers in calomel possessing linear acoustic attenuation. The formerly identified additional degree of freedom, unique to this regime, is exploited for designing the cell with an eye to doubling the resolution due to two-phonon processes. We clarify the role of varying the central acoustic frequency and acoustic attenuation using that degree of freedom. Then the efficiency of calomel is exploited to expand the cell's bandwidth with a cost of its efficiency. Proof-of-principle experiments confirm the developed approaches and illustrate their applicability to innovative techniques of optical spectrum analysis with the improved resolution. The achieved spectral resolution of 0.205 Å at 405 nm and the resolving power 19,800 are the best for acousto-optical spectrometers dedicated to space or airborne operations to date as far as we know.

  17. Band-edge optical transitions in a nonpolar-plane GaN substrate: exciton–phonon coupling and temperature effects

    NASA Astrophysics Data System (ADS)

    Wang, M. Z.; Xu, S. J.

    2016-09-01

    We present a detailed investigation of the band-edge optical transitions involving the interacting exciton–phonon system, especially first-order longitudinal optical (LO) phonon-assisted luminescence of bound and free excitons in m- and c-plane GaN substrates in a low temperature range from 4 K to 40 K. The main luminescence features of all of the three kinds of excitons can be well described by the theoretical models that take exciton-LO-phonon coupling into account. The effective Bohr radii of the excitons play a key role in determining the Huang–Rhys factor characterizing the exciton-LO-phonon coupling strength in GaN. An interesting oscillatory structure is found to appear in the low-temperature luminescence spectra of the nonpolar-plane GaN substrate, which needs to be clarified by further investigations.

  18. Ultrafast saturation of resonant optical processes

    NASA Astrophysics Data System (ADS)

    Patnaik, Anil K.; Roy, Sukesh; Gord, James R.

    2014-12-01

    A generalized formulation is presented for determining the saturation thresholds for optical processes excited by ultrafast pulses based on the pulse area of the excitation pulse. It is demonstrated that the threshold of driving-pulse intensity for absorption and fluorescence saturation in a two-level system is inversely proportional to the square of the duration of the excitation pulse. These results are obtained from both a simplified analytical solution assuming a Gaussian excitation pulse shape and a detailed numerical calculation based on density-matrix equations. The calculation is generalized further to obtain the saturation condition for a two-photon Raman process by defining a two-photon pulse area both analytically and numerically. These results not only provide predictive capabilities for determining thresholds of signal saturation using ultrashort durations with arbitrary pulse shapes and durations but also open up possibilities for predetermining the threshold intensities of various resonant nonlinear processes.

  19. Multi-coupled resonant splitting with a nano-slot metasurface and PMMA phonons

    NASA Astrophysics Data System (ADS)

    Finch, Michael F.; Lail, Brian A.

    2015-08-01

    Coupled-resonances can be used in applications that include, but are not limited to, surface-enhanced infrared spectroscopy (SEIRS), surface-enhanced Raman spectroscopy (SERS), biosensing, and index sensing. Fano resonance in analogue plasmonic systems has been described as the coupling of a bright (superradiant) mode and a dark (subradiant) mode via the near field.Dark and bright mode interactionsareinvestigated with the use of a Fano resonant metamaterial (FRMM) where the metamaterial is a dual nano-slot metasurface on a silicon cavity. The FRMM is numerically simulated using Ansys High Frequency Structure Simulator (HFSS). The FRMM is coupled to the carbon double bond in polymethyl methacrylate (PMMA) to demonstrate mode splitting and signal enhancement. Then the dual nano-slot is compared to the complementary dual nano-rod configuration.

  20. Phonon instability and self-organized structures in multilayer stacks of confined dipolar Bose-Einstein condensates in optical lattices

    NASA Astrophysics Data System (ADS)

    Köberle, Patrick; Wunner, Günter

    2009-12-01

    In calculations to date [D.-W. Wang and E. Demler, e-print arXiv:0812.1838; M. Klawunn and L. Santos, Phys. Rev. A 80, 013611 (2009)] of multilayer stacks of dipolar condensates, created in one-dimensional optical lattices, the condensates have been assumed to be two dimensional. In a real experiment, however, the condensates do not extend to infinity in the oblate direction, but have to be confined by a trap potential, too. By three-dimensional numerical simulations of this realistic experimental situation we find a crucial dependence of the phonon instability boundary on the number of layers. Moreover, near the boundary of the phonon instability, a variety of structured ground-state wave functions emerges, which may indicate the onset of a roton instability [S. Ronen, D. C. E. Bortolotti, and J. L. Bohn, Phys. Rev. Lett. 98, 030406 (2007); R. M. Wilson, S. Ronen, J. L. Bohn, and H. Pu, Phys. Rev. Lett. 100, 245302 (2008)]. We also consider the effect of a variable number of atoms per layer on the appearance of the phonon instability.

  1. Quasi-Resonant Nonlinear Absorption for Optical Power Limiting: solgel-Processed Er(3+)-Doped Multicomponent Silica Glass.

    PubMed

    Maciel, G S; Biswas, A; Friend, C S; Prasad, P N

    2000-05-20

    We demonstrate optical power limiting by what we believe to be a new mechanism of nonlinear absorption, which involves a quasi-resonant ground-state absorption that is either phonon assisted or assisted by the presence of defect sites (tail absorption). Such a mechanism provides high transmittance at low intensity yet optical limiting under cw conditions. The sample used was a novel solgel-processed Er(3+)-doped multicomponent silica glass. In this system the nonlinear absorption process is achieved because the resonant excited-state ((4)I(13/2) ? (4)S(3/2)) absorption cross section is larger than the quasi-resonant ground-state ((4)I(15/2) ? (4)I(9/2)) absorption cross section. PMID:18345156

  2. Differentiating space-time optical signals using resonant nanophotonics structures

    NASA Astrophysics Data System (ADS)

    Emelyanov, S. V.; Bykov, D. A.; Golovastikov, N. V.; Doskolovich, L. L.; Soifer, V. A.

    2016-03-01

    A theoretical description of the space-time transformations of an optical signal, which passes through resonant gratings and Bragg gratings with a defect, is proposed. The problem of differentiating a space-time optical signal using a resonant grating has been solved. The strict solution to the Maxwell equations using the Fourier modal method is involved to determine the parameters of the transfer function of the resonant diffraction structure and to carry out numerical modeling, which has confirmed the proposed theoretical description.

  3. Center mode of a doubly resonant optical periodic structure

    NASA Astrophysics Data System (ADS)

    Alagappan, G.; Png, C. E.

    2016-07-01

    An optical periodic structure with a single spatial resonance exhibits a stopband. When a second spatial resonance very close to the first one is added, the resulting doubly resonant structure exhibits a Gaussian enveloped, high quality factor transmission state right at the center of the original stopband. Using a slowly varying envelope approximation, we describe the optical characteristics of this transmission state analytically. The transmission state exists despite an optical structure of low refractive index contrast, and has potential applications in nano-optics, and photonics.

  4. How diffraction limits ultrasonic screening in phononic plate composed of a periodic array of resonant slits

    NASA Astrophysics Data System (ADS)

    Elayouch, Aliyasin; Addouche, Mahmoud; Lasaygues, Philippe; Achaoui, Younes; Ouisse, Morvan; Khelif, Abdelkrim

    2016-05-01

    We explore experimentally the role played by diffraction in the phenomenon of acoustic shielding provided by a plate that is periodically perforated with subwavelength slits and immersed in water. We carried out ultrasonic transmission measurements for all directions of propagation in order to check the omnidirectionality of acoustic shielding. While a single slit acts as a Fabry-Perot resonator in the frequency range of interest, the coupling between adjacent slits provides an attenuation frequency band centered around the resonant frequency that is mostly independent of the angle of incidence. Beyond the incident angle of 45 degrees, however, we observe the appearance of scattered radiation that limits the attenuation of ultrasound. This spurious scattering is shown to arise from diffraction by the grating of slits. xml:lang="fr"

  5. Narrow-band resonant optical reflectors and resonant optical transformers for laser stabilization and wavelength division multiplexing

    SciTech Connect

    Kazarinov, R.F.; Henry, C.H.; Olsson, N.A.

    1987-09-01

    The authors propose a new way of making highly resonant integrated optical circuits based on weak side-by-side coupling between waveguides and high Q distributed Bragg resonators. This method can be used to design a resonant optical reflector which, when used as a feedback element to a laser, will result in a compact structure that has both extremely narrow line width and very low chirp. By coupling the resonator to two waveguides, one on either side, an optical analog of the resonant transformer can be made. This device can be used for wavelength division multiplexing. Such multiplexer elements will both resonantly transform optical power from the laser to a common output channel and also provide feedback which locks the laser to the channel wavelength.

  6. Optical Fano resonance of an individual semiconductor nanostructure.

    PubMed

    Fan, Pengyu; Yu, Zongfu; Fan, Shanhui; Brongersma, Mark L

    2014-05-01

    Fano resonances with a characteristic asymmetric line shape can be observed in light scattering, transmission and reflection spectra of resonant optical systems. They result from interference between direct and indirect, resonance-assisted pathways. In the nanophotonics field, Fano effects have been observed in a wide variety of systems, including metallic nanoparticle assemblies, metamaterials and photonic crystals. Their unique properties find extensive use in applications, including optical filtering, polarization selectors, sensing, lasers, modulators and nonlinear optics. We report on the observation of a Fano resonance in a single semiconductor nanostructure, opening up opportunities for their use in active photonic devices. We also show that Fano-resonant semiconductor nanostructures afford the intriguing opportunity to simultaneously measure the far-field scattering response and the near-field energy storage by extracting photogenerated charge. Together they can provide a complete experimental characterization of this type of resonance. PMID:24747781

  7. Optical Tapers as White-Light WGM Resonators

    NASA Technical Reports Server (NTRS)

    Strekalov, Dmitry V.; Matsko, Andrey B.; Savchenkov, Anatoliy A.

    2010-01-01

    A theoretical analysis has revealed that tapered optical waveguides could be useful as white-light whispering-gallery-mode (WGM) optical resonators. The compactness and the fixed-narrow-frequency-band nature of the resonances of prior microdisk and microsphere WGM resonators are advantageous in low-power, fixed-narrow-frequency-band applications. However for optical-processing applications in which there are requirements for power levels higher and/or spectral responses broader than those of prior microdisk and microsphere WGM resonators, white-light WGM resonators in the form of optical tapers would be preferable. The theoretical analysis was performed for a multimode, axisymmetric, circular-cross-section waveguide having a taper sufficiently smooth and gradual to justify the approximation of adiabaticity. In this approximation, the equation for the dependence of the electromagnetic field upon the axial (longitudinal) waveguide coordinate can be separated from the equation for the dependence upon the radius and the azimuthal angle.

  8. Superconductivity in the two-dimensional electron gas induced by high-energy optical phonon mode and large polarization of the SrTiO3 substrate

    NASA Astrophysics Data System (ADS)

    Rosenstein, Baruch; Shapiro, B. Ya.; Shapiro, I.; Li, Dingping

    2016-07-01

    Pairing in one-atomic-layer-thick two-dimensional electron gas (2DEG) by a single flat band of high-energy longitudinal optical phonons is considered. The polar dielectric SrTiO3 (STO) exhibits such an energetic phonon mode and the 2DEG is created both when one unit cell FeSe layer is grown on its (100 ) surface and on the interface with another dielectric like LaAlO3 (LAO). We obtain a quantitative description of both systems solving the gap equation for Tc for arbitrary Fermi energy ɛF, electron-phonon coupling λ , and the phonon frequency Ω , and direct (random-phase approximation) electron-electron repulsion strength α . The focus is on the intermediate region between the adiabatic, ɛF>>Ω , and the nonadiabatic, ɛF<<Ω , regimes. The high-temperature superconductivity in single-unit-cell FeSe/STO is possible due to a combination of three factors: high-longitudinal-optical phonon frequency, large electron-phonon coupling λ ˜0.5 , and huge dielectric constant of the substrate suppression the Coulomb repulsion. It is shown that very low density electron gas in the interfaces is still capable of generating superconductivity of the order of 0.1 K in LAO/STO.

  9. Optic phonon bandwidth and lattice thermal conductivity: The case of L i2X (X =O , S, Se, Te)

    NASA Astrophysics Data System (ADS)

    Mukhopadhyay, S.; Lindsay, L.; Parker, D. S.

    2016-06-01

    We examine the lattice thermal conductivities (κl) of L i2X (X =O ,S ,Se ,Te ) using a first-principles Peierls-Boltzmann transport methodology. We find low κl values ranging between 12 and 30 W m-1K-1 despite light Li atoms, a large mass difference between constituent atoms, and tightly bunched acoustic branches, all features that give high κl in other materials including BeSe (630 W m-1K-1 ), BeTe (370 W m-1K-1 ), and cubic BAs (3170 W m-1K-1 ). Together these results suggest a missing ingredient in the basic guidelines commonly used to understand and predict κl. Unlike typical simple systems (e.g., Si, GaAs, SiC), the dominant resistance to heat-carrying acoustic phonons in L i2Se and L i2Te comes from interactions of these modes with two optic phonons. These interactions require significant bandwidth and dispersion of the optic branches, both present in L i2X materials. These considerations are important for the discovery and design of new materials for thermal management applications and give a more comprehensive understanding of thermal transport in crystalline solids.

  10. Optic phonon bandwidth and lattice thermal conductivity: The case of Li2X ( X=O , S, Se, Te)

    DOE PAGESBeta

    Mukhopadhyay, S.; Lindsay, L.; Parker, D. S.

    2016-06-07

    Here, we examine the lattice thermal conductivities ( l) of Li2X (X=O, S, Se, Te) using a first-principles Peierls-Boltzmann transport methodology. We find low l values ranging between 12 and 30 W/m-K despite light Li atoms, a large mass difference between constituent atoms and tightly bunched acoustic branches, all features that give high l in other materials including BeSe (630 W/m-1K-1), BeTe (370 W/m-1K-1) and cubic BAs (3150 W/m-1K-1). Together these results suggest a missing ingredient in the basic guidelines commonly used to understand and predict l. Unlike typical simple systems (e.g., Si, GaAs, SiC), the dominant resistance to heat-carryingmore » acoustic phonons in Li2Se and Li2Te comes from interactions of these modes with two optic phonons. These interactions require significant bandwidth and dispersion of the optic branches, both present in Li2X materials. Finally, these considerations are important for the discovery and design of new materials for thermal management applications, and give a more comprehensive understanding of thermal transport in crystalline solids.« less

  11. The effects of optical phonon on the binding energy of bound polaron in a wurtzite ZnO/Mg{sub x}Zn{sub 1–x}O quantum well

    SciTech Connect

    Zhao, Feng-Qi; Guo, Zi-Zheng; Zhu, Jun

    2014-07-07

    An improved Lee-Low-Pines intermediate coupling method is used to study the energies and binding energies of bound polarons in a wurtzite ZnO/Mg{sub x}Zn{sub 1–x}O quantum well. The contributions from different branches of long-wave optical phonons, i.e., confined optical phonons, interface optical phonons, and half-space optical phonons are considered. In addition to electron-phonon interaction, the impurity-phonon interaction, and the anisotropy of material parameters, such as phonon frequency, electron effective mass, and dielectric constant, are also included in our computation. Ground-state energies, binding energies and detailed phonon contributions from various phonons as functions of well width, impurity position and composition are presented. Our result suggests that total phonon contribution to ground state and binding energies in the studied wurtzite ZnO/Mg₀.₃Zn₀.₇O quantum wells varies between 28–23 meV and 62–45 meV, respectively, which are much larger than the corresponding values (about 3.2–1.8 meV and 1.6–0.3 meV) in GaAs/Al₀.₃Ga₀.₇As quantum wells. For a narrower quantum well, the phonon contribution mainly comes from interface and half-space phonons, for a wider quantum well, most of phonon contribution originates from confined phonons. The contribution from all the phonon modes to binding energies increases slowly either when impurity moves far away from the well center in the z direction or with the increase in magnesium composition (x). It is found that different phonons have different influences on the binding energies of bound polarons. Furthermore, the phonon contributions to binding energies as functions of well width, impurity position, and composition are very different from one another. In general, the electron-optical phonon interaction and the impurity center-optical phonon interaction play an important role in electronic states of ZnO-based quantum wells and cannot be neglected.

  12. Measurement and control of electron-phonon interactions in graphene

    NASA Astrophysics Data System (ADS)

    Remi, Sebastian

    Despite the weak interaction between electrons and atomic vibrations (phonons) in the one-atom thick crystal of carbon called graphene, the scattering of electrons off phonons limits coherent electron transport in pristine devices over mesoscopic length scales. The future of graphene as a replacement to silicon and other materials in advanced electronic devices will depend on the success of controlling and optimizing electronic transport. In this dissertation, we explore the electron-phonon interaction via Raman scattering, elucidating the effects of filling and emptying charge states on the phonons in both the metallic state and when levels are quantized by an applied perpendicular magnetic field. In zero magnetic field, the phonon energy shifts due to electronic screening by charge carriers. Previously, a logarithmic divergence of the phonon energy was predicted as a function of the charge carrier density. For the first time, we observe signatures of this logarithmic divergence at liquid He temperatures after vacuum annealing on single layers. We also measure the electron-phonon coupling strength, Fermi velocity, and broadening of electronic quantum levels from Raman scattering and correlate these parameters to electronic transport. In a strong perpendicular magnetic field, the energy bands split into discrete Landau levels. Here, we observe kinks and splitting of the optical phonon energy, even when the Landau level transitions are far from resonant with the phonons. We discover that the kinks are attributed to charge filling of Landau levels, as understood from a linearized model based on electron-phonon interactions. Moreover, we show that material parameters determined without magnetic fields also describe phonon behavior in high magnetic fields.

  13. Strain effects on the optical conductivity of gapped graphene in the presence of Holstein phonons beyond the Dirac cone approximation

    NASA Astrophysics Data System (ADS)

    Yarmohammadi, Mohsen

    2016-08-01

    In this paper we study the optical conductivity and density of states (DOS) of doped gapped graphene beyond the Dirac cone approximation in the presence of electron-phonon (e-ph) interaction under strain, i.e., within the framework of a full π-band Holstein model, by using the Kubo linear response formalism that is established upon the retarded self-energy. A new peak in the optical conductivity for a large enough e-ph interaction strength is found which is associated to transitions between the midgap states and the Van Hove singularities of the main π-band. Optical conductivity decreases with strain and at large strains, the system has a zero optical conductivity at low energies due to optically inter-band excitations through the limit of zero doping. As a result, the Drude weight changes with e-ph interaction, temperature and strain. Consequently, DOS and optical conductivity remains stable with temperature at low e-ph coupling strengths.

  14. Microwave-to-Optical Conversion in WGM Resonators

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy; Strekalov, Dmitry; Yu, Nan; Matsko, Andrey; Maleki, Lute

    2008-01-01

    Microwave-to-optical frequency converters based on whispering-gallery-mode (WGM) resonators have been proposed as mixers for the input ends of microwave receivers in which, downstream of the input ends, signals would be processed photonically. A frequency converter as proposed (see figure) would exploit the nonlinearity of the electromagnetic response of a WGM resonator made of LiNbO3 or another suitable ferroelectric material. Up-conversion would take place by three-wave mixing in the resonator. The WGM resonator would be de - signed and fabricated to obtain (1) resonance at both the microwave and the optical operating frequencies and (2) phase matching among the input and output microwave and optical signals as described in the immediately preceding article. Because the resonator would be all dielectric there would be no metal electrodes signal losses would be very low and, consequently, the resonance quality factors (Q values) of the microwave and optical fields would be very large. The long lifetimes associated with the large Q values would enable attainment of high efficiency of nonlinear interaction with low saturation power. It is anticipated that efficiency would be especially well enhanced by the combination of optical and microwave resonances in operation at input signal frequencies between 90 and 300 GHz.

  15. Uniaxial strain-induced Kohn anomaly and electron-phonon coupling in acoustic phonons of graphene

    NASA Astrophysics Data System (ADS)

    Cifuentes-Quintal, M. E.; de la Peña-Seaman, O.; Heid, R.; de Coss, R.; Bohnen, K.-P.

    2016-08-01

    Recent advances in strain engineering at the nanoscale have shown the feasibility to modulate the properties of graphene. Although the electron-phonon (e-ph) coupling and Kohn anomalies in graphene define the phonon branches contributing to the resonance Raman scattering and are relevant to the electronic and thermal transport as a scattering source, the evolution of the e-ph coupling as a function of strain has been less studied. In this work, the Kohn anomalies and the e-ph coupling in uniaxially strained graphene along armchair and zigzag directions were studied by means of density functional perturbation theory calculations. In addition to the phonon anomaly at the transversal optical (TO) phonon branch in the K point for pristine graphene, we found that uniaxial strain induces a discontinuity in the frequency derivative of the longitudinal acoustic phonon branch. This behavior corresponds to the emergence of a Kohn anomaly, as a consequence of a strain-enhanced e-ph coupling. Thus, the present results for uniaxially strained graphene contrast with the commonly assumed view that the e-ph coupling around the K point is only present in the TO phonon branch.

  16. Anomalous Phonon Dispersion of an Ultracold - Mixture in a Square Optical Lattice

    NASA Astrophysics Data System (ADS)

    Koinov, Zlatko; Pahl, Shanna; Mendoza, Rafael

    2015-05-01

    A necessary condition for the damping of the long-wavelength excitations of the superfluid phase (referred to as superfluid phonons) due to the three-particle process is to have an anomalous phonon dispersion. The existence of anomalous phonon dispersion has been confirmed in superfluid . There are no experimental data suggesting that this phenomenon exists in superfluid Fermi gases. To the best of our knowledge, the existence of anomalous dispersion has been theoretically predicted only in atomic spin balanced Fermi gas close to the unitarity limit. The numerical results reported here suggest that the anomalous long-wavelength dispersion can be realized in mass and spin imbalanced atomic Fermi gases away from the unitary limit. In particular, the numerical solution of the Bethe-Salpeter equation in a weak-coupling regime shows that the long-wavelength part of the collective-mode dispersion of the superfluid Fulde-Ferrell phase of a mixture of population-imbalanced Lithium-6 and Potassium-40 atoms in a square lattice at some values of polarization, interacting strength and temperature initially bends upward before bending over.

  17. Resonant microwave cavity for 8.5-12 GHz optically detected electron spin resonance with simultaneous nuclear magnetic resonance

    NASA Astrophysics Data System (ADS)

    Colton, J. S.; Wienkes, L. R.

    2009-03-01

    We present a newly developed microwave resonant cavity for use in optically detected magnetic resonance (ODMR) experiments. The cylindrical quasi-TE011 mode cavity is designed to fit in a 1 in. magnet bore to allow the sample to be optically accessed and to have an adjustable resonant frequency between 8.5 and 12 GHz. The cavity uses cylinders of high dielectric material, so-called "dielectric resonators," in a double-stacked configuration to determine the resonant frequency. Wires in a pseudo-Helmholtz configuration are incorporated into the cavity to provide frequencies for simultaneous nuclear magnetic resonance (NMR). The system was tested by measuring cavity absorption as microwave frequencies were swept, by performing ODMR on a zinc-doped InP sample, and by performing optically detected NMR on a GaAs sample. The results confirm the suitability of the cavity for ODMR with simultaneous NMR.

  18. WGM Resonators for Terahertz-to-Optical Frequency Conversion

    NASA Technical Reports Server (NTRS)

    Strekalov,Dmitry; Savchenkov, Anatoliy; Matsko, Andrey; Nu, Nan

    2008-01-01

    Progress has been made toward solving some practical problems in the implementation of terahertz-to-optical frequency converters utilizing whispering-gallery-mode (WGM) resonators. Such frequency converters are expected to be essential parts of non-cryogenic terahertz- radiation receivers that are, variously, under development or contemplated for a variety of applications in airborne and spaceborne instrumentation for astronomical and military uses. In most respects, the basic principles of terahertz-to-optical frequency conversion in WGM resonators are the same as those of microwave (sub-terahertz)-to-optical frequency conversion in WGM resonators, various aspects of which were discussed in the three preceeding articles. To recapitulate: In a receiver following this approach, a preamplified incoming microwave signal (in the present case, a terahertz signal) is up-converted to an optical signal by a technique that exploits the nonlinearity of the electromagnetic response of a whispering-gallery-mode (WGM) resonator made of LiNbO3 or another suitable electro-optical material. Upconversion takes place by three-wave mixing in the resonator. To ensure the required interaction among the optical and terahertz signals, the WGM resonator must be designed and fabricated to function as an electro-optical modulator while simultaneously exhibiting (1) resonance at the required microwave and optical operating frequencies and (2) phase matching among the microwave and optical signals circulating in the resonator. Downstream of the WGM resonator, the up-converted signal is processed photonically by use of a tunable optical filter or local oscillator and is then detected. The practical problems addressed in the present development effort are the following: Satisfaction of the optical and terahertz resonance-frequency requirement is a straightforward matter, inasmuch as the optical and terahertz spectra can be measured. However, satisfaction of the phase-matching requirement is

  19. All-optical scheme for detecting the possible Majorana signature based on QD and nanomechanical resonator systems

    NASA Astrophysics Data System (ADS)

    Chen, HuaJun; Zhu, KaDi

    2015-05-01

    Majorana fermions (MFs) are exotic particles that are their own anti-particles. Currently, the search for MFs occurring as quasiparticle excitations in condensed matter systems has attracted widespread interest, because of their importance in fundamental physics and potential applications in topological quantum computation based on solid-state devices. Motivated by recent experimental progress towards the detection and manipulation of MFs in hybrid semiconductor/superconductor heterostructures, in this review, we present a novel proposal to probe MFs in all-optical domain. We introduce a single quantum dot (QD), a hybrid quantum dot-nanomechanical resonators (QD-NR) system, and a carbon nanotube (CNT) resonator implanted in a single electron spin system with optical pump-probe technology to detect MFs, respectively. With this scheme, a possible Majorana signature is investigated via the probe absorption spectrum and nonlinear optical Kerr effect, and the coupling strength between MFs and the QD or the single electron spin is also determined. In the hybrid QD-NR system, vibration of the NR will enhance the nonlinear optical effect, which makes the MFs more sensitive for detection. In the CNT resonator with a single electron, the single electron spin can be considered as a sensitive probe, and the CNT resonator behaved as a phonon cavity is robust for detecting of MFs. This optical scheme will provide another method for the detection MFs and will open the door for new applications ranging from robust manipulation of MFs to quantum information processing based on MFs.

  20. Nonlinear optics and crystalline whispering gallery mode resonators

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey; Savchenkov, Anatoliy; Ilchenko, Vladimir S.; Maleki, Lute

    2004-01-01

    We report on our recent results concerning fabrication of high-Q whispering gallery mode crystalline resonaors, and discuss some possible applications of lithium niobate WGM resonators in nonlinear optics and photonics.

  1. Analysis of an integrated optic micro racetrack resonator based biosensor

    NASA Astrophysics Data System (ADS)

    Malathi, S.; Hegde, Gopalkrishna; Srinivas, T.; Roy, Ugra M.

    2014-06-01

    Silicon-On- Insulator (SOI) technology has huge potential in fabricating compact devices for various applications such as integrated optic waveguides, directional couplers, resonators etc. In this work, we present the analysis of a biosensor based on an integrated optic racetrack resonator, interrogated by a bus waveguide. The biomaterial is applied as a cladding layer. Here we analyze the coupling between the resonator and the bus waveguide, and its dependence on the bio layer. In traditional analysis, the effective refractive index and resonator total path length are the factors influencing the resonant wavelength. Our analysis shows that all parametric values decrease with increase in waveguide width and spacing. The inclusion of waveguide mode overlap and perturbation in coupled mode equation results in enhanced resonator sensitivity of an order of magnitude

  2. Whispering Gallery Optical Resonator Spectroscopic Probe and Method

    NASA Technical Reports Server (NTRS)

    Anderson, Mark S. (Inventor)

    2014-01-01

    Disclosed herein is a spectroscopic probe comprising at least one whispering gallery mode optical resonator disposed on a support, the whispering gallery mode optical resonator comprising a continuous outer surface having a cross section comprising a first diameter and a second diameter, wherein the first diameter is greater than the second diameter. A method of measuring a Raman spectrum and an Infra-red spectrum of an analyte using the spectroscopic probe is also disclosed.

  3. White-Light Whispering-Gallery-Mode Optical Resonators

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey; Savchenkov, Anatoliy; Maleki, Lute

    2006-01-01

    Whispering-gallery-mode (WGM) optical resonators can be designed to exhibit continuous spectra over wide wavelength bands (in effect, white-light spectra), with ultrahigh values of the resonance quality factor (Q) that are nearly independent of frequency. White-light WGM resonators have potential as superior alternatives to (1) larger, conventional optical resonators in ring-down spectroscopy, and (2) optical-resonator/electro-optical-modulator structures used in coupling of microwave and optical signals in atomic clocks. In these and other potential applications, the use of white-light WGM resonators makes it possible to relax the requirement of high-frequency stability of lasers, thereby enabling the use of cheaper lasers. In designing a white-light WGM resonator, one exploits the fact that the density of the mode spectrum increases predictably with the thickness of the resonator disk. By making the resonator disk sufficiently thick, one can make the frequency differences between adjacent modes significantly less than the spectral width of a single mode, so that the spectral peaks of adjacent modes overlap, making the resonator spectrum essentially continuous. Moreover, inasmuch as the Q values of the various modes are determined primarily by surface Rayleigh scattering that does not depend on mode numbers, all the modes have nearly equal Q. By use of a proper coupling technique, one can ensure excitation of a majority of the modes. For an experimental demonstration of a white-light WGM resonator, a resonator disk 0.5-mm thick and 5 mm in diameter was made from CaF2. The shape of the resonator and the fiberoptic coupling arrangement were as shown in Figure 1. The resonator was excited with laser light having a wavelength of 1,320 nm and a spectral width of 4 kHz. The coupling efficiency exceeded 80 percent at any frequency to which the laser could be set in its tuning range, which was >100-GHz wide. The resonator response was characterized by means of ring

  4. Quantum correlations among optical and vibrational quanta

    NASA Astrophysics Data System (ADS)

    Carlig, Sergiu; Macovei, Mihai A.

    2014-05-01

    We investigate the feasibility of correlating an optical cavity field and a vibrational phonon mode. A laser pumped quantum dot fixed on a nanomechanical resonator beam interacts as a whole with the optical resonator mode. When the quantum dot variables are faster than the optical and phonon ones, we obtain a final master equation describing the involved modes only. Increasing the temperature, which directly affects the vibrational degrees of freedom, one can as well influence the cavity photon intensity, i.e., the optical and phonon modes are correlated. Furthermore, the corresponding Cauchy-Schwarz inequality is violated demonstrating the quantum nature of those correlations.

  5. Integrated resonant micro-optical gyroscope and method of fabrication

    DOEpatents

    Vawter, G. Allen; Zubrzycki, Walter J.; Guo, Junpeng; Sullivan, Charles T.

    2006-09-12

    An integrated optic gyroscope is disclosed which is based on a photonic integrated circuit (PIC) having a bidirectional laser source, a pair of optical waveguide phase modulators and a pair of waveguide photodetectors. The PIC can be connected to a passive ring resonator formed either as a coil of optical fiber or as a coiled optical waveguide. The lasing output from each end of the bidirectional laser source is phase modulated and directed around the passive ring resonator in two counterpropagating directions, with a portion of the lasing output then being detected to determine a rotation rate for the integrated optical gyroscope. The coiled optical waveguide can be formed on a silicon, glass or quartz substrate with a silicon nitride core and a silica cladding, while the PIC includes a plurality of III V compound semiconductor layers including one or more quantum well layers which are disordered in the phase modulators and to form passive optical waveguides.

  6. Isotropically sensitive optical filter employing atomic resonance transitions

    DOEpatents

    Marling, John B.

    1981-01-01

    An ultra-high Q isotropically sensitive optical filter or optical detector employing atomic resonance transitions. More specifically, atomic resonance transitions utilized in conjunction with two optical bandpass filters provide an optical detector having a wide field of view (.about.2.pi. steradians) and very narrow acceptance bandwidth approaching 0.01 A. A light signal to be detected is transmitted through an outer bandpass filter into a resonantly absorbing atomic vapor, the excited atomic vapor then providing a fluorescence signal at a different wavelength which is transmitted through an inner bandpass filter. The outer and inner bandpass filters have no common transmission band, thereby resulting in complete blockage of all optical signals that are not resonantly shifted in wavelength by the intervening atomic vapor. Two embodiments are disclosed, one in which the light signal raises atoms contained in the atomic vapor from the ground state to an excited state from which fluorescence occurs, and the other in which a pump laser is used to raise the atoms in the ground state to a first excited state from which the light signal then is resonantly absorbed, thereby raising the atoms to a second excited state from which fluorescence occurs. A specific application is described in which an optical detector according to the present invention can be used as an underwater detector for light from an optical transmitter which could be located in an orbiting satellite.

  7. On the path length of an excess electron interacted with optical phonons in a molecular chain

    NASA Astrophysics Data System (ADS)

    Lakhno, V. D.

    2008-08-01

    We show that in a molecular chain with dispersionless phonons at zero temperature, a “quasistationary” moving soliton state of an excess electron is possible. As the soliton velocity vanishes, the path length of the excess electron exponentially tends to infinity. It is demonstrated that in the presence of dispersion, when the soliton initial velocity exceeds the maximum group velocity of the chain, the soliton slows down until it reaches the maximum group velocity and then moves stationarily at this maximum group velocity. A conclusion is made of the fallacy of some works were the existence of moving polarons in a dispersionless medium is considered infeasible.

  8. Experimental study on resonator micro-optic gyroscope

    NASA Astrophysics Data System (ADS)

    Zhao, Meng; Shi, Bang-ren; Chen, Chen; Guo, Li-jun; Zhang, Rong; Zhang, Qiu-e.

    2011-08-01

    Resonator optic gyroscope (ROG) based on Sagnac effect has been investigated over the past years and developed as an attractive device for many applications. Resonator micro-optic gyroscope (R-MOG) with an only several-cm-long ring on a wafer is a promising candidate for the new generation inertial rotation sensor. Using micro machining process, R-MOG was manufactured on the silicon or LiNbO3 wafer by etching passive optical ring resonator devices. It has great advantages by realizing the minitype. R-MOG is a kind of optic gyroscope by detecting the resonance frequency difference of the clockwise and counterclockwise resonance to measure the angular velocity. The Sagnac effect is extremely weak, so the detection method has been the key point in researching R-MOG. Using the multi-beam superposition principle, we theoretically analyzed the signal detection scheme based on laser frequency modulation and experimentally investigated the equivalent open-loop signals of a R-MOG chip. The passive ring resonator (PRR), the core component of R-MOG, was composed of a ring waveguide with a radius of 2cm and an optical coupler with the coupling ratio of 12%. The resonance curve showed that the free spectral range (FSR), full width at half maximum (FWHM) and fineness were 3.0378GHz, 74.09MHz and 41, respectively. In the equivalent open-loop experiment, the counterclockwise (CCW) light frequency was locked to its resonant point, and the clockwise (CW) optical frequency changed around the CW resonant point. The experimental results illustrated that the sensitivity of the R-MOG was 6.15 rad/s.

  9. Coherence Phenomena in Coupled Optical Resonators

    NASA Technical Reports Server (NTRS)

    Smith, D. D.; Chang, H.

    2004-01-01

    We predict a variety of photonic coherence phenomena in passive and active coupled ring resonators. Specifically, the effective dispersive and absorptive steady-state response of coupled resonators is derived, and used to determine the conditions for coupled-resonator-induced transparency and absorption, lasing without gain, and cooperative cavity emission. These effects rely on coherent photon trapping, in direct analogy with coherent population trapping phenomena in atomic systems. We also demonstrate that the coupled-mode equations are formally identical to the two-level atom Schrodinger equation in the rotating-wave approximation, and use this result for the analysis of coupled-resonator photon dynamics. Notably, because these effects are predicted directly from coupled-mode theory, they are not unique to atoms, but rather are fundamental to systems of coherently coupled resonators.

  10. One-shot calculation of temperature-dependent optical spectra and phonon-induced band-gap renormalization

    NASA Astrophysics Data System (ADS)

    Zacharias, Marios; Giustino, Feliciano

    2016-08-01

    Recently, Zacharias et al. [Phys. Rev. Lett. 115, 177401 (2015), 10.1103/PhysRevLett.115.177401] developed an ab initio theory of temperature-dependent optical absorption spectra and band gaps in semiconductors and insulators. In that work, the zero-point renormalization and the temperature dependence were obtained by sampling the nuclear wave functions using a stochastic approach. In the present work, we show that the stochastic sampling of Zacharias et al. can be replaced by fully deterministic supercell calculations based on a single optimal configuration of the atomic positions. We demonstrate that a single calculation is able to capture the temperature-dependent band-gap renormalization including quantum nuclear effects in direct-gap and indirect-gap semiconductors, as well as phonon-assisted optical absorption in indirect-gap semiconductors. In order to demonstrate this methodology, we calculate from first principles the temperature-dependent optical absorption spectra and the renormalization of direct and indirect band gaps in silicon, diamond, and gallium arsenide, and we obtain good agreement with experiment and with previous calculations. In this work we also establish the formal connection between the Williams-Lax theory of optical transitions and the related theories of indirect absorption by Hall, Bardeen, and Blatt, and of temperature-dependent band structures by Allen and Heine. The present methodology enables systematic ab initio calculations of optical absorption spectra at finite temperature, including both direct and indirect transitions. This feature will be useful for high-throughput calculations of optical properties at finite temperature and for calculating temperature-dependent optical properties using high-level theories such as G W and Bethe-Salpeter approaches.

  11. Generation of Coherent Phonons in a CdTe Single Crystal Using an Ultrafast Two-Phonon Laser-Excitation Process

    NASA Astrophysics Data System (ADS)

    Mizoguchi, K.; Morishita, R.; Oohata, G.

    2013-02-01

    The detection-energy dependence of a coherent phonon in a (001) CdTe crystal, generated by ultrashort laser pulses with the center energy transparent or opaque to the sample, is investigated using a spectrally resolved pump-probe method. At the excitation in the transparent region, the detection-energy dependence of the phonon amplitude has two peaks at the energy shifted by one times the phonon energy of CdTe from the center energy of the probe pulses. On the other hand, the amplitude in the opaque region shows two peaks at the energy shifted by about two times the phonon energy. This difference occurs even though the observed energies of the coherent phonons in both regions are the same as that of the longitudinal optical phonon of CdTe. The energy shifts in the detection-energy dependence imply that the emission and absorption of one phonon and two phonons in the transparent and opaque regions, respectively, are implicated in coherent phonon generation. In this study, the detection-energy dependence is examined from the viewpoint of the third-order nonlinear susceptibility based on the impulsive stimulated Raman scattering process under nonresonant and resonant conditions.

  12. On-chip microfluidic tuning of an optical microring resonator

    NASA Astrophysics Data System (ADS)

    Levy, Uriel; Campbell, Kyle; Groisman, Alex; Mookherjea, Shayan; Fainman, Yeshaiahu

    2006-03-01

    We describe the design, fabrication, and operation of a tunable optical filter based on a bus waveguide coupled to a microring waveguide resonator located inside a microchannel in a microfluidic chip. Liquid flowing in the microchannel constitutes the upper cladding of the waveguides. The refractive index of the liquid controls the resonance wavelengths and strength of coupling between the bus waveguide and the resonator. The refractive index is varied by on-chip mixing of two source liquids with different refractive indices. We demonstrate adjustment of the resonance by 2nm and tuning the filter to an extinction ratio of 37dB.

  13. Isotropically sensitive optical filter employing atomic resonance transitions

    DOEpatents

    Marling, J.B.

    An ultra-high Q isotropically sensitive optical filter or optical detector is disclosed employing atomic resonance transitions. More specifically, atomic resonance transitions utilized in conjunction with two optical bandpass filters provide an optical detector having a wide field of view (approx. 2 ..pi.. steradians) and very narrow acceptance bandwidth approaching 0.01A. A light signal to be detected is transmitted through an outer bandpass filter into a resonantly absorbing atomic vapor, the excited atomic vapor than providing a fluorescence signal at a different wavelength which is transmitted through an inner bandpass filters have no common transmission band, therby resulting in complete blockage of all optical signals that are not resonantly shifted in wavelength by the intervening atomic vapor. Two embodiments are disclosed, one in which the light signal raises atoms contained in the atomic vapor from the ground state to an excited state from which fluorescence occurs, and the other in which a pump laser is used to raise the atoms in the ground state to a first excited state from which the light signal then is resonantly absorbed, thereby raising the atoms to a second excited state from which fluorescence occurs. A specific application is described in which an optical detector according to the present invention can be located in an orbiting satellite.

  14. GHz spurious mode free AlN lamb wave resonator with high figure of merit using one dimensional phononic crystal tethers

    NASA Astrophysics Data System (ADS)

    Wu, Guoqiang; Zhu, Yao; Merugu, Srinivas; Wang, Nan; Sun, Chengliang; Gu, Yuandong

    2016-07-01

    This letter reports a spurious mode free GHz aluminum nitride (AlN) lamb wave resonator (LWR) towards high figure of merit (FOM). One dimensional gourd-shape phononic crystal (PnC) tether with large phononic bandgaps is employed to reduce the acoustic energy dissipation into the substrate. The periodic PnC tethers are based on a 1 μm-thick AlN layer with 0.26 μm-thick Mo layer on top. A clean spectrum over a wide frequency range is obtained from the measurement, which indicates a wide-band suppression of spurious modes. Experimental results demonstrate that the fabricated AlN LWR has an insertion loss of 5.2 dB and a loaded quality factor (Q) of 1893 at 1.02 GHz measured in air. An impressive ratio of the resistance at parallel resonance (Rp) to the resistance at series resonance (Rs) of 49.8 dB is obtained, which is an indication of high FOM for LWR. The high Rp to Rs ratio is one of the most important parameters to design a radio frequency filter with steep roll-off.

  15. Optically pumped subwavelength-scale metallodielectric nanopatch resonators.

    PubMed

    Kwon, Kyungmok; You, Jong-Bum; Shim, Jaeho; Jung, Youngho; Yu, Kyoungsik

    2016-01-01

    We discuss subwavelength-scale semiconductor metal-optic resonators placed on the metal substrate with various top metal plate sizes. Albeit with large optical losses, addition of metal layers converts a leaky semiconductor nano-block into a highly-confined optical cavity. Optically pumped lasing action is observed with the extended top metal layer that can significantly suppress the radiation losses. Careful investigation of self-heating effects during the optical carrier injection process shows the importance of temperature-dependent material properties in the laser rate equation model and the overall laser performances. PMID:27549640

  16. Magnetic resonance imaging of the optic nerves and chiasm

    SciTech Connect

    Daniels, D.L.; Herfkins, R.; Gager, W.E.; Meyer, G.A.; Koehler, P.R.; Williams, A.L.; Haughton, V.M.

    1984-07-01

    Magnetic resonance imaging (MR) of the optic nerves and chiasm was compared with computed tomography (CT) in 4 healthy volunteers, 4 patients without orbital or chiasmal abnormalities, and 4 patients with tumor (anterior clinoid meningioma in 2, optic nerve glioma in 1, and optic nerve sheath meningioma in 1). MR was found to be effective in demonstrating the optic nerves and related structures, particularly the intracanalicular portion of the nerve which is difficult to see with CT. Best results were achieved with partial saturation recovery (SR) images. As axial views cannot always distinguish the ethmoid sinus tissue from the optic nerve, it may be necessary to employ both axial and coronal images.

  17. Optically pumped subwavelength-scale metallodielectric nanopatch resonators

    PubMed Central

    Kwon, Kyungmok; You, Jong-bum; Shim, Jaeho; Jung, Youngho; Yu, Kyoungsik

    2016-01-01

    We discuss subwavelength-scale semiconductor metal-optic resonators placed on the metal substrate with various top metal plate sizes. Albeit with large optical losses, addition of metal layers converts a leaky semiconductor nano-block into a highly-confined optical cavity. Optically pumped lasing action is observed with the extended top metal layer that can significantly suppress the radiation losses. Careful investigation of self-heating effects during the optical carrier injection process shows the importance of temperature-dependent material properties in the laser rate equation model and the overall laser performances. PMID:27549640

  18. Far-Field Spectroscopy and Near-Field Optical Imaging of Coupled Plasmon-Phonon Polaritons in 2D van der Waals Heterostructures.

    PubMed

    Yang, Xiaoxia; Zhai, Feng; Hu, Hai; Hu, Debo; Liu, Ruina; Zhang, Shunping; Sun, Mengtao; Sun, Zhipei; Chen, Jianing; Dai, Qing

    2016-04-01

    A new hybridized plasmon-phonon polariton mode in graphene/h-BN van der Waals heterostructures is presented, featuring the ultrahigh field confinement characteristic of the graphene plasmon and the long lifetime property of the h-BN transverse optical phonon. This enables an ultralong hybrid plasmon lifetime of up to 1.6 ps (with ultrahigh mode confinement up to >l0 (2) /7000 and ultrasmall group velocity down to 0.001c, where c is the speed of light in vacuum), superior to any localized plasmon ever demonstrated. PMID:26889663

  19. Effect of Longitudinal Optical Phonon--Plasmon Coupling on the Transient Self-Consistent Field in GaAs p--i--n Diodes

    NASA Astrophysics Data System (ADS)

    Thao, Dinh Nhu; The, Nguyen Phuoc

    2013-10-01

    The effect of longitudinal optical (LO) phonon--coherent plasmon coupling on the transient self-consistent field and then on frequency spectra of collective oscillations in GaAs p--i--n diodes without a biased field is investigated by the self-consistent ensemble Monte Carlo method. The frequency spectra of collective oscillations in the diodes show that there are two new strong peaks in the terahertz range when the coupling is taken into account. These peaks replace the coupled phonon--plasmon peaks in the bulk semiconductor.

  20. Mueller matrix ellipsometry studies of the optical phonons and crystal field excitations in multiferroic orthoferrites RFeO3 (R=Tb,Dy)

    NASA Astrophysics Data System (ADS)

    Martinez, V. A.; Stanislavchuk, T. N.; Sirenko, A. A.; Litvinchuk, A. P.; Wang, Yazhong; Cheong, S. W.

    Optical properties of multiferroic orthoferrites RFeO3 (R=Tb,Dy) bulk crystals have been studied in the far-infrared range from 50 to 1000 cm-1 and temperatures from 7 K to 300 K. Mueller matrix and rotating analyzer ellipsometry measurements were carried out at the U4IR beamline of the National Synchrotron Light Source at Brookhaven National Lab. Optical phonon spectra and crystal field excitations were measured for all three orthorhombic axes of RFeO3. In the experimental temperature dependencies of the phonon frequencies we found non-Grüneisen behavior caused by the electron-phonon and spin-phonon interactions. We determined the symmetries and selection rules for the crystal field transitions in Tb3+ and Dy3+ ions. Magnetic field dependencies of the optical spectra allowed us to determine anisotropy of the crystal field g-factors for Tb3+ and Dy3+ ions. This Project is supported by collaborative DOE Grant DE-FG02-07ER46382 between Rutgers U. and NJIT. Use of NSLS-BNL was supported by DOE DE-AC02-98CH10886. V.A. Martinez was supported by NEU NSF-1343716.

  1. Raman scattering by confined optical phonons in Si and Ge nanostructures.

    PubMed

    Alfaro, Pedro; Cisneros, Rodolfo; Bizarro, Monserrat; Cruz-Irisson, Miguel; Wang, Chumin

    2011-03-01

    A microscopic theory of the Raman scattering based on the local bond-polarizability model is presented and applied to the analysis of phonon confinement in porous silicon and porous germanium, as well as nanowire structures. Within the linear response approximation, the Raman shift intensity is calculated by means of the displacement-displacement Green's function and the Born model, including central and non-central interatomic forces. For the porous case, the supercell method is used and ordered pores are produced by removing columns of Si or Ge atoms from their crystalline structures. This microscopic theory predicts a remarkable shift of the highest-frequency of first-order Raman peaks towards lower energies, in comparison with the crystalline case. This shift is discussed within the quantum confinement framework and quantitatively compared with the experimental results obtained from porous silicon samples, which were produced by anodizing p--type (001)-oriented crystalline Si wafers in a hydrofluoric acid bath. PMID:21270988

  2. Optical Probing of Ultrafast Electronic Decay in Bi and Sb with Slow Phonons

    NASA Astrophysics Data System (ADS)

    Li, J. J.; Chen, J.; Reis, D. A.; Fahy, S.; Merlin, R.

    2013-01-01

    Illumination with laser sources leads to the creation of excited electronic states of particular symmetries, which can drive isosymmetric vibrations. Here, we use a combination of ultrafast stimulated and cw spontaneous Raman scattering to determine the lifetime of A1g and Eg electronic coherences in Bi and Sb. Our results both shed new light on the mechanisms of coherent phonon generation and represent a novel way to probe extremely fast electron decoherence rates. The Eg state, resulting from an unequal distribution of carriers in three equivalent band regions, is extremely short lived. Consistent with theory, the lifetime of its associated driving force reaches values as small as 2 (6) fs for Bi (Sb) at 300 K.

  3. Demonstration of sharp multiple Fano resonances in optical metamaterials.

    PubMed

    Moritake, Yuto; Kanamori, Yoshiaki; Hane, Kazuhiro

    2016-05-01

    We experimentally demonstrated multiple Fano resonances in optical metamaterials. By combination of two different sized asymmetric-double-bar (ADB) structures, triple Fano resonance was observed in the near-infrared region. In addition to Fano resonance due to anti-phase modes in isolated ADB structures, an anti-phase mode due to coupling among different sized ADBs was observed. Dependence of characteristics of resonances on size difference was also investigated. At specific conditions of size difference, quality factors of three Fano resonances were improved compared with ADB metamaterials consisting of one kind of ADBs. The results will help to realize applications using metamaterial resonators with multiple functionalities and high performance. PMID:27137549

  4. Optical Twist Induced by Plasmonic Resonance

    NASA Astrophysics Data System (ADS)

    Chen, Jun; Wang, Neng; Cui, Liyong; Li, Xiao; Lin, Zhifang; Ng, Jack

    2016-06-01

    Harvesting light for optical torque is of significant importance, owing to its ability to rotate nano- or micro-objects. Nevertheless, applying a strong optical torque remains a challenging task: angular momentum must conserve but light is limited. A simple argument shows the tendency for two objects with strong mutual scattering or light exchange to exhibit a conspicuously enhanced optical torque without large extinction or absorption cross section. The torque on each object is almost equal but opposite, which we called optical twist. The effect is quite significant for plasmonic particle cluster, but can also be observed in structures with other morphologies. Such approach exhibits an unprecedentedly large torque to light extinction or absorption ratio, enabling limited light to exert a relatively large torque without severe heating. Our work contributes to the understanding of optical torque and introduces a novel way to manipulate the internal degrees of freedom of a structured particle cluster.

  5. Optical Twist Induced by Plasmonic Resonance

    PubMed Central

    Chen, Jun; Wang, Neng; Cui, Liyong; Li, Xiao; Lin, Zhifang; Ng, Jack

    2016-01-01

    Harvesting light for optical torque is of significant importance, owing to its ability to rotate nano- or micro-objects. Nevertheless, applying a strong optical torque remains a challenging task: angular momentum must conserve but light is limited. A simple argument shows the tendency for two objects with strong mutual scattering or light exchange to exhibit a conspicuously enhanced optical torque without large extinction or absorption cross section. The torque on each object is almost equal but opposite, which we called optical twist. The effect is quite significant for plasmonic particle cluster, but can also be observed in structures with other morphologies. Such approach exhibits an unprecedentedly large torque to light extinction or absorption ratio, enabling limited light to exert a relatively large torque without severe heating. Our work contributes to the understanding of optical torque and introduces a novel way to manipulate the internal degrees of freedom of a structured particle cluster. PMID:27291860

  6. Optical Twist Induced by Plasmonic Resonance.

    PubMed

    Chen, Jun; Wang, Neng; Cui, Liyong; Li, Xiao; Lin, Zhifang; Ng, Jack

    2016-01-01

    Harvesting light for optical torque is of significant importance, owing to its ability to rotate nano- or micro-objects. Nevertheless, applying a strong optical torque remains a challenging task: angular momentum must conserve but light is limited. A simple argument shows the tendency for two objects with strong mutual scattering or light exchange to exhibit a conspicuously enhanced optical torque without large extinction or absorption cross section. The torque on each object is almost equal but opposite, which we called optical twist. The effect is quite significant for plasmonic particle cluster, but can also be observed in structures with other morphologies. Such approach exhibits an unprecedentedly large torque to light extinction or absorption ratio, enabling limited light to exert a relatively large torque without severe heating. Our work contributes to the understanding of optical torque and introduces a novel way to manipulate the internal degrees of freedom of a structured particle cluster. PMID:27291860

  7. Resonance damping and optical susceptibilities (Critical Review Lecture)

    NASA Astrophysics Data System (ADS)

    Andrews, David L.; Davila Romero, Luciana C.

    2003-07-01

    In the formal development of optical response theory in terms of susceptibilities, proper representation of the optical frequency dependence necessitates modeling both the discrete linewidth and the finite signal enhancement associated with the onset of resonance. Such dispersion behavior is generally accommodated by damping factors, featured in both resonant and non-resonant susceptibility terms. For the resonant terms, the sign of such damping corrections is unequivocal; however the correct choice of sign for non-resonant terms has become a matter of debate, heightened by the discovery that entirely opposite conventions are applied in mainstream literature on Raman scattering and nonlinear optics. Where the two conventions are applied to electro-optical processes in fluids there are significant and potentially verifiable differences between the associated results. Through a full thorough quantum electrodynamical treatment the universal correctness of one convention can be ascertained and flaws in the counter-convention identified. Resolution of the central issue requires consideration of a number of fundamental questions concerning the nature of dissipation in quantum mechanical systems. It is concluded that optical susceptibilities formulated with correct signing of the damping corrections must fulfill several fundamental tests: satisfaction of a new sum rule; invariance of the associated quantum amplitudes under time-reversal symmetry, and a resilience to canonical transformation.

  8. Improving the Optical Quality Factor of the WGM Resonator

    NASA Technical Reports Server (NTRS)

    Savchenkov, Anatoliy; Matsko, Andrey; Iltchenko, Vladimir

    2008-01-01

    Resonators usually are characterized with two partially dependent values: finesse (F) and quality factor (Q). The finesse of an empty Fabry-Perot (FP) resonator is defined solely by the quality of its mirrors and is calculated as F=piR(exp 1/2)/(1-R). The maximum up-to-date value of reflectivity R approximately equal to 1 - 1.6 x 10(exp -6) is achieved with dielectric mirrors. An FP resonator made with the mirrors has finesse F=1.9 x 10(exp 6). Further practical increase of the finesse of FP resonators is problematic because of the absorption and the scattering of light in the mirror material through fundamental limit on the reflection losses given by the internal material losses and by thermodynamic density fluctuations on the order of parts in 109. The quality factor of a resonator depends on both its finesse and its geometrical size. A one-dimensional FP resonator has Q=2 F L/lambda, where L is the distance between the mirrors and lambda is the wavelength. It is easy to see that the quality factor of the resonator is unlimited because L is unlimited. F and Q are equally important. In some cases, finesse is technically more valuable than the quality factor. For instance, buildup of the optical power inside the resonator, as well as the Purcell factor, is proportional to finesse. Sometimes, however, the quality factor is more valuable. For example, inverse threshold power of intracavity hyperparametric oscillation is proportional to Q(exp 2) and efficiency of parametric frequency mixing is proportional to Q(exp 3). Therefore, it is important to know both the maximally achievable finesse and quality factor values of a resonator. Whispering gallery mode (WGM) resonators are capable of achieving larger finesse compared to FP resonators. For instance, fused silica resonators with finesse 2.3 x 10(exp 6) and 2.8 x 10(exp 6) have been demonstrated. Crystalline WGM resonators reveal even larger finesse values, F=6.3 x 10(exp 6), because of low attenuation of light in the

  9. Interplay between low-energy optical phonon modes and structural transition in PrT2Zn20 (T=Ru and Ir)

    NASA Astrophysics Data System (ADS)

    Wakiya, K.; Onimaru, T.; Tsutsui, S.; Matsumoto, K. T.; Nagasawa, N.; Baron, A. Q. R.; Hasegawa, T.; Ogita, N.; Udagawa, M.; Takabatake, T.

    2015-03-01

    Atomic dynamics of PrT2Zn20 for T=Ru with a structural transition at Ts=138 K and T=Ir without such a transition have been studied by inelastic X-ray scattering (IXS) measurements. The IXS spectra for T=Ru reveal an optical phonon excitation at 3 meV. We assign it to low-energy vibration of the Zn atom at the 16c site by taking account of the first principles calculation [Hasegawa et al. 2012 J. Phys.: Conf. Proc. 391 012016]. For T=Ir, on the other hand, the optical excitation at 3 meV was not observed. The contrasting results indicate that the low-energy optical phonon mode has a role in the structural transition in PrRu2Zn20 and isostructural La counterparts.

  10. Optical biosensors using surface plasmon resonance

    NASA Astrophysics Data System (ADS)

    Homola, Jiri; Brynda, Eduard; Tobiska, Petr; Tichy, Ivo; Skvor, Jiri

    1999-12-01

    We present a surface plasmon resonance sensor base on prism excitation of surface plasmons and spectral interrogation. For specific detection of biomolecular analytes, multilayers of monoclonal antibodies are immobilized on the surface of the sensor. Detection of biomolecular analytes such as human (beta) -2)-microglobulin, choriogonadotropin, hepatitis B surface antigen, salmonella enteritidis is demonstrated.

  11. Digital crossbar switch using nonlinear optical ring resonator

    NASA Astrophysics Data System (ADS)

    McAulay, Alastair D.

    2009-08-01

    Optical elements are preferred to electronic ones for military computing and communications to reduce vulnerability to electromagnetic pulses from nuclear explosion, electromagnetic bombs or lightning. Equations are derived for an optical micro ring resonator and for a nonlinear ring resonator that uses Kerr material so that the resonant frequency changes with light intensity in the ring. The switch can be modulated at faster than 10 Gbps for compatibility with electronic switches and equipment. A two-by-two switch is described based on the nonlinear ring resonator. A Benes network is constructed using the two-by-two switches. This allows full permutations of the inputs by means of an algorithm for setting the switches. Several rings are used for each frequency with slightly different frequencies to allow switching of wavelength division multiplexed signals.

  12. Optical trapping of dielectric nanoparticles in resonant cavities

    SciTech Connect

    Hu Juejun; Lin Shiyun; Crozier, Kenneth; Kimerling, Lionel C.

    2010-11-15

    We theoretically investigate the opto-mechanical interactions between a dielectric nanoparticle and the resonantly enhanced optical field inside a high Q, small-mode-volume optical cavity. We develop an analytical method based on open system analysis to account for the resonant perturbation due to particle introduction and predict trapping potential in good agreement with three-dimensional (3D) finite-difference time-domain (FDTD) numerical simulations. Strong size-dependent trapping dynamics distinctly different from free-space optical tweezers arise as a consequence of the finite cavity perturbation. We illustrate single nanoparticle trapping from an ensemble of monodispersed particles based on size-dependent trapping dynamics. We further discover that the failure of the conventional dipole approximation in the case of resonant cavity trapping originates from a new perturbation interaction mechanism between trapped particles and spatially localized photons.

  13. Resonant diffraction gratings for spatial differentiation of optical beams

    SciTech Connect

    Golovastikov, N V; Bykov, D A; Doskolovich, L L

    2014-10-31

    Diffraction of a two-dimensional optical beam from a resonant diffraction grating is considered. It is shown that at certain resonance parameters the diffraction grating allows for spatial differentiation and integration of the incident beam. The parameters of the diffraction grating for spatial differentiation of optical beams in the transmission geometry are calculated. It is shown that the differentiating diffraction grating allows the conversion of the two-dimensional beam into the two-dimensional Hermite – Gaussian mode. The presented results of numerical modelling are in good agreement with the proposed theoretical description. The use of the considered resonant diffraction gratings is promising for solving the problems of all-optical data processing. (laser applications and other topics in quantum electronics)

  14. Nonreciprocal optical properties in resonant hybrid photonic crystals

    NASA Astrophysics Data System (ADS)

    D'Andrea, A.; Tomassini, N.

    2016-07-01

    The present work is devoted to the theoretical study of the nonreciprocal optical properties in hybrid (isotropic and anisotropic) periodic multilayers for photon energy values chosen close to the electronic energy gaps of semiconductors (excitons). The optical properties of these resonant nonmagnetic photonic crystals, where linear and quadratic spatial dispersion effects are both present, will be studied in the framework of exciton-polariton self-consistent solutions of the Maxwell and Schrödinger equations in the effective-mass approximation. The main interesting optical properties, namely, giant transmission, absorption suppression, and optical unidirectional propagation, will be computed by implementing a two-layer "minimum model."

  15. Observation of optical bistability due to resonator configuration transition

    NASA Astrophysics Data System (ADS)

    Lee, C. S.; Osada, H.

    1985-05-01

    In this Letter, a new kind of active optical bistability is discussed. The basic principle underlying the operation of the optically bistable laser is based on stable-unstable cavity configuration transitions of an active optical resonator. Generally speaking, a laser system showing both pump- and laser-induced lensing (focusing or defocusing) effects may display such a hysteresis loop in its input-output characteristics. This bistability is experimentally demonstrated using a flashlamp-pumped, Nd-doped gadolinium gallium garnet rod placed in a plane-parallel optical cavity.

  16. Optical chiral metamaterial based on the resonant behaviour of nanodiscs

    NASA Astrophysics Data System (ADS)

    Kordi, Mahdi; Mojtaba Mirsalehi, Mir

    2016-08-01

    Circular dichorism and optical activity have been achieved by chiral metamaterials in the optical spectrum, but for the case of negative index of refraction, remarkable achievements have not been obtained in this region so far. We employ nanoparticles to shift the resonant frequency of a chiral metamaterial based on twisted cross wires to optical domain. Our proposed structure provides giant optical activity, strong circular dichorism and also negative refractive index in the optical wavelengths. Optical activity in our structure has a rotary power similar to a gyrotropic crystal of quartz, but in a thickness which is four orders of magnitude smaller. The foundation of our method for realizing such an optical chiral metamaterial is based on creating a different coupling between longitudinal modes of localized surface plasmons for right and left circularly polarized incident waves.

  17. Waveguide ring resonator as integrated optics for rotation sensor

    NASA Astrophysics Data System (ADS)

    Tang, Quan'an; Zheng, Ludi; Ma, Xinyu; Zhang, Yanshen

    1996-09-01

    To obtain a micro optic rotation sensor (MORS), a passive ring resonator (PRR) based on channel waveguide was designed and investigated. The waveguide structure of the resonator includes a ring waveguide as well as two directional couplers. The theoretical resolution and transfer functions of the MORS are discussed, and the PRR parameters are determined. According to the sensitivity requirement, the PRR frequency detecting system is discussed, and different detecting schemes are compared.

  18. Label-Free Optical Ring Resonator Bio/Chemical Sensors

    NASA Astrophysics Data System (ADS)

    Zhu, Hongying; Suter, Jonathan D.; Fan, Xudong

    Optical micro-ring resonator sensors are an emerging category of label-free optical sensors for bio/chemical sensing that have recently been under intensive investigation. Researchers of this technology have been motivated by a tremendous breadth of different applications, including medical diagnosis, environmental monitoring, homeland security, and food quality control, which require sensitive analytical tools. Ring resonator sensors use total internal reflection to support circulating optical resonances called whispering gallery modes (WGMs). The WGMs have an evanescent field of several hundred nanometers into the surrounding medium, and can therefore detect the refractive index change induced when the analyte binds to the resonator surface. Despite the small physical size of a resonator, the circulating nature of the WGM creates extremely long effective lengths, greatly increasing light-matter interaction and improving its sensing performance. Moreover, only small sample volume is needed for detection because the sensors can be fabricated in sizes well below 100 μm. The small footprint allows integration of those ring resonator sensors onto lab-on-a-chip types of devices for multiplexed detection.

  19. A study of non-equilibrium phonons in GaAs/AlAs quantum wells

    SciTech Connect

    Su, Zhenpeng

    1996-11-01

    In this thesis we have studied the non-equilibrium phonons in GaAs/AlAs quantum wells via Raman scattering. We have demonstrated experimentally that by taking into account the time-reversal symmetry relation between the Stokes and anti-Stokes Raman cross sections, one can successfully measure the non-equilibrium phonon occupancy in quantum wells. Using this technique, we have studied the subject of resonant intersubband scattering of optical phonons. We find that interface roughness plays an important role in resonant Raman scattering in quantum wells. The lateral size of the smooth regions in such interface is estimated to be of the order of 100 {Angstrom}. Through a study of photoluminescence of GaAs/AlAs quantum wells under high intensity laser excitation, we have found that band nonparabolicity has very little effect on the electron subband energies even for subbands as high as a few hundred meV above the lowest one. This finding may require additional theoretical study to understand its origin. We have also studied phonon confinement and propagation in quantum wells. We show that Raman scattering of non-equilibrium phonons in quantum wells can be a sensitive measure of the spatial extent of the longitudinal optical (LO) phonons. We deduce the coherence length of LO phonons in GaAs/Al{sub x}Ga{sub 1-x}As quantum wells as a function of the Al concentration x.

  20. Transformation optics with Fabry-Pérot resonances

    NASA Astrophysics Data System (ADS)

    Sadeghi, M. M.; Li, Sucheng; Xu, Lin; Hou, Bo; Chen, Huanyang

    2015-03-01

    Transformation optics is a powerful tool to design various novel devices, such as invisibility cloak. Fantastic effects from this technique are usually accompanied with singular mappings, resulting in challenging implementations and narrow bands of working frequencies. Here in this article, Fabry-Pérot resonances in materials of extreme anisotropy are used to design various transformation optical devices that are not only easy to realize but also work well for a set of resonant frequencies (multiple frequencies). As an example, a prototype of a cylindrical concentrator is fabricated for microwaves.

  1. Transformation optics with Fabry-Pérot resonances

    PubMed Central

    Sadeghi, M. M.; Li, Sucheng; Xu, Lin; Hou, Bo; Chen, Huanyang

    2015-01-01

    Transformation optics is a powerful tool to design various novel devices, such as invisibility cloak. Fantastic effects from this technique are usually accompanied with singular mappings, resulting in challenging implementations and narrow bands of working frequencies. Here in this article, Fabry-Pérot resonances in materials of extreme anisotropy are used to design various transformation optical devices that are not only easy to realize but also work well for a set of resonant frequencies (multiple frequencies). As an example, a prototype of a cylindrical concentrator is fabricated for microwaves. PMID:25726924

  2. Optical properties of MgZnO alloys: Excitons and exciton-phonon complexes

    SciTech Connect

    Neumann, M. D.; Cobet, C.; Esser, N.; Laumer, B.; Wassner, T. A.; Eickhoff, M.; Feneberg, M.; Goldhahn, R.

    2011-07-01

    The characteristics of the excitonic absorption and emission around the fundamental bandgap of wurtzite Mg{sub x}Zn{sub 1-x}O grown on c-plane sapphire substrates by plasma assisted molecular beam epitaxy with Mg contents between x = 0 and x = 0.23 are studied using spectroscopic ellipsometry and photoluminescence (PL) measurements. The ellipsometric data were analyzed using a multilayer model yielding the dielectric function (DF). The imaginary part of the DF for the alloys exhibits a pronounced feature which is attributed to exciton-phonon coupling (EPC) similar to the previously reported results for ZnO. Thus, in order to determine reliable transition energies, the spectral dependence is analyzed by a model which includes free excitonic lines, the exciton continuum, and the enhanced absorption due to EPC. A line shape analysis of the temperature-dependent PL spectra yielded in particular the emission-related free excitonic transition energies, which are compared to the results from the DF line-shape analysis. The PL linewidth is discussed within the framework of an alloy disorder model.

  3. Magnetic Resonance Reversals in Optically Pumped Alkali-Metal Vapor

    NASA Astrophysics Data System (ADS)

    Gong, Fei; Jau, Yuan-Yu; Happer, William

    2007-06-01

    We report an unusual new phenomenon, peculiar sign reversals of the ground-state magnetic resonances and of the ``zero-dip" resonance (Zeeman resonance at zero field) of optically-pumped, alkali-metal vapors. These anomalies occur when a ``weak" circular polarized D1 laser light is tuned to pump atoms predominantly from the lower ground-state hyperfine multiplet. One can understand the signal reversals in simple, semi-quantitative way with reference to this distribution. uantitative computer simulations are in excellent greement with observations.

  4. Magnetic resonance reversals in optically pumped alkali-metal vapor

    NASA Astrophysics Data System (ADS)

    Gong, F.; Jau, Y.-Y.; Happer, W.

    2007-05-01

    We report an unusual phenomenon, peculiar sign reversals of the ground-state magnetic resonances and of the zero-dip resonance (Zeeman resonance at zero field) of optically pumped, alkali-metal vapors. These anomalies occur when a weak circularly polarized D1 laser light is tuned to pump atoms predominantly from the lower ground-state hyperfine multiplet. One can understand the signal reversals in a simple, semiquantitative way with reference to the spin-temperature distribution. Quantitative computer simulations are in excellent agreement with observations.

  5. Optical Fiber Excitation of Fano Resonances in a Silicon Microsphere

    NASA Astrophysics Data System (ADS)

    Sabahattin Gökay, Ulaş; Zakwan, Muhammad; Demir, Abdullah; Serpengüzel, Ali

    2016-01-01

    In this article, Fano lineshape whispering gallery modes were observed in the light scattering spectrum of a silicon microsphere in near-infrared telecommunication wavelengths. A simple model is presented to explain the transition from Lorentzian lineshape to the Fano lineshape resonances with the coupled-mode theory of multiple whispering gallery modes. Polar mode spacing of 0.23 nm is observed in the spectra, which correlates well with the calculated value. The quality factor of the Lorentzian and Fano resonances are on the order of 105. By using an appropriate interface design for the microsphere coupling geometries, Fano lineshape optical resonances herald novel device applications for silicon volumetric lightwave circuits.

  6. Optically driven resonance of nanoscale flexural oscillators in liquid.

    PubMed

    Verbridge, Scott S; Bellan, Leon M; Parpia, Jeevak M; Craighead, H G

    2006-09-01

    We demonstrate the operation of radio frequency nanoscale flexural resonators in air and liquid. Doubly clamped string, as well as singly clamped cantilever resonators, with nanoscale cross-sectional dimensions and resonant frequencies as high as 145 MHz are driven in air as well as liquid with an amplitude modulated laser. We show that this laser drive technique can impart sufficient energy to a nanoscale resonator to overcome the strong viscous damping present in these media, resulting in a mechanical resonance that can be measured by optical interference techniques. Resonance in air, isopropyl alcohol, acetone, water, and phosphate-buffered saline is demonstrated for devices having cross-sectional dimensions close to 100 nm. For operation in air, quality factors as high as 400 at 145 MHz are demonstrated. In liquid, quality factors ranging from 3 to 10 and frequencies ranging from 20 to 100 MHz are observed. These devices, and an all-optical actuation and detection system, may provide insight into the physics of the interaction of nanoscale mechanical structures with their environments, greatly extending the viscosity range over which such small flexural resonant devices can be operated. PMID:16968035

  7. Phonons and electron-phonon interaction in halogen-fullerene compounds

    NASA Astrophysics Data System (ADS)

    Limonov, M. F.; Kitaev, Yu. E.; Chugreev, A. V.; Smirnov, V. P.; Grushko, Yu. S.; Kolesnik, S. G.; Kolesnik, S. N.

    1998-04-01

    We have investigated the optical spectra of different halogen-fullerene compounds: C60I4-x, C70I2, C60Br24, C60Cl24, and C70Cl17. Two types of carbon-halogen bonding have been established: (a) C60I4-x and C70I2 compounds are formed by a C60 or C70 molecule sublattice and an I2 molecule sublattice that weakly interact via van der Waals forces; (b) C60Br24, C60Cl24, and C70Cl17 compounds are characterized by covalent bonds between C and Br/Cl atoms. We have studied in detail the resonance effects in C60Cl24 using the methods of Raman scattering, infrared absorption, and absorption in the visible region. The effect originates from the interactions between the phonon subsystem and the electron band at 2.33 eV and manifests itself in a resonant enhancement of the Raman line intensities and in the repetition of the phonon and the luminescence spectra shifted by the frequency of Raman-active phonon at 1508 cm-1. The group-theory analysis of phonon symmetries in rigid and nonrigid C60Br24 and C60Cl24 crystals has been performed.

  8. Applications of Optical Microcavity Resonators in Analytical Chemistry

    NASA Astrophysics Data System (ADS)

    Wade, James H.; Bailey, Ryan C.

    2016-06-01

    Optical resonator sensors are an emerging class of analytical technologies that use recirculating light confined within a microcavity to sensitively measure the surrounding environment. Bolstered by advances in microfabrication, these devices can be configured for a wide variety of chemical or biomolecular sensing applications. We begin with a brief description of optical resonator sensor operation, followed by discussions regarding sensor design, including different geometries, choices of material systems, methods of sensor interrogation, and new approaches to sensor operation. Throughout, key developments are highlighted, including advancements in biosensing and other applications of optical sensors. We discuss the potential of alternative sensing mechanisms and hybrid sensing devices for more sensitive and rapid analyses. We conclude with our perspective on the future of optical microcavity sensors and their promise as versatile detection elements within analytical chemistry.

  9. Quantum field theory of interacting plasmon-photon-phonon system

    NASA Astrophysics Data System (ADS)

    Hieu Nguyen, Van; Nguyen, Bich Ha

    2015-09-01

    This work is devoted to the construction of the quantum field theory of the interacting system of plasmons, photons and phonons on the basis of general fundamental principles of electrodynamics and quantum field theory of many-body systems. Since a plasmon is a quasiparticle appearing as a resonance in the collective oscillation of the interacting electron gas in solids, the starting point is the total action functional of the interacting system comprising electron gas, electromagnetic field and phonon fields. By means of the powerful functional integral technique, this original total action is transformed into that of the system of the quantum fields describing plasmons, transverse photons, acoustic as well as optic longitudinal and transverse phonons. The collective oscillations of the electron gas is characterized by a real scalar field φ(x) called the collective oscillation field. This field is split into the static background field φ0(x) and the fluctuation field ζ(x). The longitudinal phonon fields {{{Q}}al}(x), {{{Q}}ol}(x) are also split into the background fields {Q}0al(x), {Q}0ol(x) and dynamical fields {{{q}}al}(x), {{{q}}ol}(x) while the transverse phonon fields {{{Q}}at}(x), {{{Q}}ot}(x) themselves are dynamical fields {{{q}}at}(x), {{{q}}ot}(x) without background fields. After the canonical quantization procedure, the background fields φ0(x), {Q}0al(x), {Q}0ol(x) remain the classical fields, while the fluctuation fields ζ(x) and dynamical phonon fields {{{q}}al}(x), {{{q}}at}(x), {{{q}}ol}(x), {{{q}}ot}(x) become quantum fields. In quantum theory, a plasmon is the quantum of Hermitian scalar field σ(x) called the plasmon field, longitudinal phonons as complex spinless quasiparticles are the quanta of the effective longitudinal phonon Hermitian scalar fields {{θ }a}(x), {{θ }0}(x), while transverse phonons are the quanta of the original Hermitian transverse phonon vector fields {{{q}}at}(x), {{{q}}ot}(x). By means of the functional integral

  10. Steady-state linear optical properties and Kerr nonlinear optical response of a four-level quantum dot with phonon-assisted transition

    NASA Astrophysics Data System (ADS)

    Yan-Chao, She; Ting-Ting, Luo; Wei-Xi, Zhang; Mao-Wu, Ran; Deng-Long, Wang

    2016-01-01

    The linear optical properties and Kerr nonlinear optical response in a four-level loop configuration GaAs/AlGaAs semiconductor quantum dot are analytically studied with the phonon-assisted transition (PAT). It is shown that the changes among a single electromagnetically induced transparency (EIT) window, a double EIT window and the amplification of the probe field in the absorption curves can be controlled by varying the strength of PAT κ. Meanwhile, double switching from the anomalous dispersion regime to the normal dispersion regime can likely be achieved by increasing the Rabi energy of the external optical control field. Furthermore, we demonstrate that the group velocity of the probe field can be practically regulated by varying the PAT and the intensity of the optical control field. In the nonlinear case, it is shown that the large SPM and XPM can be achieved as linear absorption vanishes simultaneously, and the PAT can suppress both third-order self-Kerr and the cross-Kerr nonlinear effect of the QD. Our study is much more practical than its atomic counterpart due to its flexible design and the controllable interference strength, and may provide some new possibilities for technological applications. Project supported by the National Natural Science Foundation of China (Grant No. 61367003), the Scientific Research Fund of Hunan Provincial Education Department, China (Grant No. 12A140), and the Scientific Research Fund of Guizhou Provincial Education Department, China (Grant Nos. KY[2015]384 and KY[2015]446).

  11. Spin microscope based on optically detected magnetic resonance

    SciTech Connect

    Berman, Gennady P.; Chernobrod, Boris M.

    2009-11-10

    The invention relates to scanning magnetic microscope which has a photoluminescent nanoprobe implanted in the tip apex of an atomic force microscope (AFM), a scanning tunneling microscope (STM) or a near-field scanning optical microscope (NSOM) and exhibits optically detected magnetic resonance (ODMR) in the vicinity of impaired electron spins or nuclear magnetic moments in the sample material. The described spin microscope has demonstrated nanoscale lateral resolution and single spin sensitivity for the AFM and STM embodiments.

  12. Spin microscope based on optically detected magnetic resonance

    SciTech Connect

    Berman, Gennady P.; Chernobrod, Boris M.

    2010-06-29

    The invention relates to scanning magnetic microscope which has a photoluminescent nanoprobe implanted in the tip apex of an atomic force microscope (AFM), a scanning tunneling microscope (STM) or a near-field scanning optical microscope (NSOM) and exhibits optically detected magnetic resonance (ODMR) in the vicinity of unpaired electron spins or nuclear magnetic moments in the sample material. The described spin microscope has demonstrated nanoscale lateral resolution and single spin sensitivity for the AFM and STM embodiments.

  13. Spin microscope based on optically detected magnetic resonance

    SciTech Connect

    Berman, Gennady P.; Chernobrod, Boris M.

    2010-07-13

    The invention relates to scanning magnetic microscope which has a photoluminescent nanoprobe implanted in the tip apex of an atomic force microscope (AFM), a scanning tunneling microscope (STM) or a near-field scanning optical microscope (NSOM) and exhibits optically detected magnetic resonance (ODMR) in the vicinity of unpaired electron spins or nuclear magnetic moments in the sample material. The described spin microscope has demonstrated nanoscale lateral resolution and single spin sensitivity for the AFM and STM embodiments.

  14. Spin microscope based on optically detected magnetic resonance

    SciTech Connect

    Berman, Gennady P.; Chernobrod, Boris M.

    2009-10-27

    The invention relates to scanning magnetic microscope which has a photoluminescent nanoprobe implanted in the tip apex of an atomic force microscope (AFM), a scanning tunneling microscope (STM) or a near-field scanning optical microscope (NSOM) and exhibits optically detected magnetic resonance (ODMR) in the vicinity of unpaired electron spins or nuclear magnetic moments in the sample material. The described spin microscope has demonstrated nanoscale lateral resolution and single spin sensitivity for the AFM and STM embodiments.

  15. Spin microscope based on optically detected magnetic resonance

    DOEpatents

    Berman, Gennady P.; Chernobrod, Boris M.

    2007-12-11

    The invention relates to scanning magnetic microscope which has a photoluminescent nanoprobe implanted in the tip apex of an atomic force microscope (AFM), a scanning tunneling microscope (STM) or a near-field scanning optical microscope (NSOM) and exhibits optically detected magnetic resonance (ODMR) in the vicinity of unpaired electron spins or nuclear magnetic moments in the sample material. The described spin microscope has demonstrated nanoscale lateral resolution and single spin sensitivity for the AFM and STM embodiments.

  16. Squeezing Alters Frequency Tuning of WGM Optical Resonator

    NASA Technical Reports Server (NTRS)

    Mohageg, Makan; Maleki, Lute

    2010-01-01

    Mechanical squeezing has been found to alter the frequency tuning of a whispering-gallery-mode (WGM) optical resonator that has an elliptical shape and is made of lithium niobate. It may be possible to exploit this effect to design reconfigurable optical filters for optical communications and for scientific experiments involving quantum electrodynamics. Some background information is prerequisite to a meaningful description of the squeezing-induced alteration of frequency tuning: The spectrum of a WGM resonator is represented by a comblike plot of intensity versus frequency. Each peak of the comblike plot corresponds to an electromagnetic mode represented by an integer mode number, and the modes are grouped into sets represented by integer mode indices. Because lithium niobate is an electro-optically active material, the WGM resonator can be tuned (that is, the resonance frequencies can be shifted) by applying a suitable bias potential. The frequency shift of each mode is quantified by a tuning rate defined as the ratio between the frequency shift and the applied potential. In the absence of squeezing, all modes exhibit the same tuning rate. This concludes the background information. It has been demonstrated experimentally that when the resonator is squeezed along part of either of its two principal axes, tuning rates differ among the groups of modes represented by different indices (see figure). The differences in tuning rates could be utilized to configure the resonance spectrum to obtain a desired effect; for example, through a combination of squeezing and electrical biasing, two resonances represented by different mode indices could be set at a specified frequency difference something that could not be done through electrical biasing alone.

  17. Critical Coupling Between Optical Fibers and WGM Resonators

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey; Maleki, Lute; Itchenko, Vladimir; Savchenkov, Anatoliy

    2009-01-01

    Two recipes for ensuring critical coupling between a single-mode optical fiber and a whispering-gallery-mode (WGM) optical resonator have been devised. The recipes provide for phase matching and aperture matching, both of which are necessary for efficient coupling. There is also a provision for suppressing intermodal coupling, which is detrimental because it drains energy from desired modes into undesired ones. According to one recipe, the tip of the single-mode optical fiber is either tapered in diameter or tapered in effective diameter by virtue of being cleaved at an oblique angle. The effective index of refraction and the phase velocity at a given position along the taper depend on the diameter (or effective diameter) and the index of refraction of the bulk fiber material. As the diameter (or effective diameter) decreases with decreasing distance from the tip, the effective index of refraction also decreases. Critical coupling and phase matching can be achieved by placing the optical fiber and the resonator in contact at the proper point along the taper. This recipe is subject to the limitation that the attainable effective index of refraction lies between the indices of refraction of the bulk fiber material and the atmosphere or vacuum to which the resonator and fiber are exposed. The other recipe involves a refinement of the previously developed technique of prism coupling, in which the light beam from the optical fiber is collimated and focused onto one surface of a prism that has an index of refraction greater than that of the resonator. Another surface of the prism is placed in contact with the resonator. The various components are arranged so that the collimated beam is focused at the prism/resonator contact spot. The recipe includes the following additional provisions:

  18. SU-F-BRE-12: Optical Resonator Water Calorimeter

    SciTech Connect

    Abraham, J; DeMarco, J; Low, D

    2014-06-15

    Purpose: Water calorimetry based on resistance thermometry has matured as a primary standard. Developing an optical technique hold the promise to push the boundaries of what is currently achievable with dosimetry. We will present a feasibility study and the current progress of construction of a Fabry-Perot resonator for dose to water measurement. Additionally, estimations of the theoretical limits resonator sensitivity and potential sources of noise for the system are described. Methods: A temperature change from the dose to water would be measured by the change in the index of refraction from the water in the cavity. Calculations are presented of the expected signal from the resonator for dose to water. The Fabry-Perot resonator constructed from optical quality narrowband mirrors is described. A water cell will be inserted into the cavity gap to provide the medium swept cavity length technique is explored as a specific implementation of this technique. Results: Calculations indicate that a dose to water on the order of a Gray is measureable with a reasonably implementable system. A resonator is currently under construction and progress towards a proof of principle measurement will be presented. The primary sources of noise, in order of importance, are expected to be; optical absorption by the medium, mechanical perturbations of the cavity length and thermal expansion of the optical mounts. Estimations of these noise sources and mitigation techniques will be discussed. Conclusion: A Fabry-Perot resonator is a promising technique for measuring the absorbed dose to water from a radiotherapy beam. This technique has the potential to serve as a check on the current primary standard for dose to water measurements. As well, i0074 may be the foundation for a new class of optical property based dosimetry measurement.

  19. Optic Nerve Assessment Using 7-Tesla Magnetic Resonance Imaging

    PubMed Central

    Singh, Arun D.; Platt, Sean M.; Lystad, Lisa; Lowe, Mark; Oh, Sehong; Jones, Stephen E.; Alzahrani, Yahya; Plesec, Thomas

    2016-01-01

    Purpose The purpose of this study was to correlate high-resolution magnetic resonance imaging (MRI) and histologic findings in a case of juxtapapillary choroidal melanoma with clinical evidence of optic nerve invasion. Methods With institutional review board approval, an enucleated globe with choroidal melanoma and optic nerve invasion was imaged using a 7-tesla MRI followed by histopathologic evaluation. Results Optical coherence tomography, B-scan ultrasonography, and 1.5-tesla MRI of the orbit (1-mm sections) could not detect optic disc invasion. Ex vivo, 7-tesla MRI detected optic nerve invasion, which correlated with histopathologic features. Conclusions Our case demonstrates the potential to document the existence of optic nerve invasion in the presence of an intraocular tumor, a feature that has a major bearing on decision making, particularly for consideration of enucleation. PMID:27239461

  20. Optical Fano resonances in a nonconcentric nanoshell.

    PubMed

    Norton, Stephen J; Vo-Dinh, Tuan

    2016-04-01

    The interaction of light with a metal nanoshell with an off-center core generates multipoles of all orders. We show here that the matrix elements used to compute the multipole expansion coefficients can be derived analytically and, with this result, we can show explicitly how the dipole and quadrupole terms in the expansion are coupled and give rise to a Fano resonance. We also show that the off-center core significantly increases the electric field enhancement at the shell surface compared to the concentric case, which can be exploited for surface-enhanced sensing. The multipole solutions are confirmed with finite-element calculations. PMID:27139663

  1. Manipulation of thermal phonons

    NASA Astrophysics Data System (ADS)

    Hsu, Chung-Hao

    Developing materials that can conduct electricity easily, but block the motion of phonons is necessary in the applications of thermoelectric devices, which can generate electricity from temperature differences. In converse, a key requirement as chips get faster is to obtain better ways to dissipate heat. Controlling heat transfer in these crystalline materials devices --- such as silicon --- is important. The heat is actually the motion or vibration of atoms known as phonons. Finding ways to manipulate the behavior of phonons is crucial for both energy applications and the cooling of integrated circuits. A novel class of artificially periodic structured materials --- phononic crystals --- might make manipulation of thermal phonons possible. In many fields of physical sciences and engineering, acoustic wave propagation in solids attracts many researchers. Wave propagation phenomena can be analyzed by mathematically solving the acoustic wave equation. However, wave propagation in inhomogeneous media with various geometric structures is too complex to find an exact solution. Hence, the Finite Difference Time Domain method is developed to investigate these complicated problems. In this work, the Finite-Difference Time-Domain formula is derived from acoustic wave equations based on the Taylor's expansion. The numerical dispersion and stability problems are analyzed. In addition, the convergence conditions of numerical acoustic wave are stated. Based on the periodicity of phononic crystal, the Bloch's theorem is applied to fulfill the periodic boundary condition of the FDTD method. Then a wide-band input signal is used to excite various acoustic waves with different frequencies. In the beginning of the calculation process, the wave vector is chosen and fixed. By means of recording the displacement field and taking the Fourier transformation, we can obtain the eigenmodes from the resonance peaks of the spectrum and draw the dispersion relation curve of acoustic waves

  2. Measurements of the Electric Field of Zero-Point Optical Phonons in GaAs Quantum Wells Support the Urbach Rule for Zero-Temperature Lifetime Broadening

    NASA Astrophysics Data System (ADS)

    Bhattacharya, Rupak; Mondal, Richarj; Khatua, Pradip; Rudra, Alok; Kapon, Eli; Malzer, Stefan; Döhler, Gottfried; Pal, Bipul; Bansal, Bhavtosh

    2015-01-01

    We study a specific type of lifetime broadening resulting in the well-known exponential "Urbach tail" density of states within the energy gap of an insulator. After establishing the frequency and temperature dependence of the Urbach edge in GaAs quantum wells, we show that the broadening due to the zero-point optical phonons is the fundamental limit to the Urbach slope in high-quality samples. In rough analogy with Welton's heuristic interpretation of the Lamb shift, the zero-temperature contribution to the Urbach slope can be thought of as arising from the electric field of the zero-point longitudinal-optical phonons. The value of this electric field is experimentally measured to be 3 kV cm-1 , in excellent agreement with the theoretical estimate.

  3. Reconfigurable Optical Spectra from Perturbations on Elliptical Whispering Gallery Resonances

    NASA Technical Reports Server (NTRS)

    Mohageg, Makan; Maleki, Lute

    2008-01-01

    Elastic strain, electrical bias, and localized geometric deformations were applied to elliptical whispering-gallery-mode resonators fabricated with lithium niobate. The resultant perturbation of the mode spectrum is highly dependant on the modal indices, resulting in a discretely reconfigurable optical spectrum. Breaking of the spatial degeneracy of the whispering-gallery modes due to perturbation is also observed.

  4. Ultra-sensitive thermometer based on a compact optical resonator

    PubMed Central

    Weng, Wenle; Luiten, Andre N

    2014-01-01

    This article demonstrates a thermometer based on millimeter-scale crystalline disk optical-resonator. By measuring the relative speed difference between 2 colors of light that travel inside the disk, the temperature changes of the disk was measured with a precision of 30 billionths of a degree. PMID:27226990

  5. Spatiotemporal optical pulse transformation by a resonant diffraction grating

    SciTech Connect

    Golovastikov, N. V.; Bykov, D. A. Doskolovich, L. L. Soifer, V. A.

    2015-11-15

    The diffraction of a spatiotemporal optical pulse by a resonant diffraction grating is considered. The pulse diffraction is described in terms of the signal (the spatiotemporal incident pulse envelope) passage through a linear system. An analytic approximation in the form of a rational function of two variables corresponding to the angular and spatial frequencies has been obtained for the transfer function of the system. A hyperbolic partial differential equation describing the general form of the incident pulse envelope transformation upon diffraction by a resonant diffraction grating has been derived from the transfer function. A solution of this equation has been obtained for the case of normal incidence of a pulse with a central frequency lying near the guided-mode resonance of a diffraction structure. The presented results of numerical simulations of pulse diffraction by a resonant grating show profound changes in the pulse envelope shape that closely correspond to the proposed theoretical description. The results of the paper can be applied in creating new devices for optical pulse shape transformation, in optical information processing problems, and analog optical computations.

  6. Reconfigurable optical spectra from perturbations on elliptical whispering gallery resonances.

    PubMed

    Mohageg, Makan; Maleki, Lute

    2008-02-01

    Elastic strain, electrical bias, and localized geometric deformations were applied to elliptical whispering-gallery-mode resonators fabricated with lithium niobate. The resultant perturbation of the mode spectrum is highly dependant on the modal indices, resulting in a discretely reconfigurable optical spectrum. Breaking of the spatial degeneracy of the whispering-gallery modes due to perturbation is also observed. PMID:18542283

  7. Spinning optical resonator sensor for torsional vibrational applications measurements

    NASA Astrophysics Data System (ADS)

    Ali, Amir R.; Gatherer, Andrew; Ibrahim, Mariam S.

    2016-03-01

    Spinning spherical resonators in the torsional vibrational applications could cause a shift in its whispering gallery mode (WGM). The centripetal force acting on the spinning micro sphere resonator will leads to these WGM shifts. An analysis and experiment were carried out in this paper to investigate and demonstrate this effect using different polymeric resonators. In this experiment, centripetal force exerted by the DC-Motor on the sphere induces an elastic deformation of the resonator. This in turn induces a shift in the whispering gallery modes of the sphere resonator. Materials used for the sphere are polydimethylsiloxane (PDMS 60:1 where 60 parts base silicon elastomer to 1 part polymer curing agent by volume) with shear modulus (G≍1kPa), (PDMS 10:1) with shear modulus (G≍300kPa), polymethylmethacrylate (PMMA, G≍2.6×109GPa) and silica (G≍3×1010 GPa). The sphere size was kept constant with 1mm in diameter for all above materials. The optical modes of the sphere exit using a tapered single mode optical fiber that is coupled to a distributed feedback laser. The transmission spectrum through the fiber is monitored to detect WGM shifts. The results showed the resonators with smaller shear modulus G experience larger WGM shift due to the larger mechanical deformation induced by the applied external centripetal force. Also, the results show that angular velocity sensors used in the torsional vibrational applications could be designed using this principle.

  8. Optical control of Magnetic Feshbach Resonances using Closed Channel EIT

    NASA Astrophysics Data System (ADS)

    Jagannathan, Arunkumar; Arunkumar, Nithya; Joseph, James; Thomas, John

    2016-05-01

    Optical techniques can provide rapid temporal control and high-resolution spatial control of interactions in cold gases enabling the study of non-equilibrium strongly interacting Fermi gases. We use electromagnetically induced transparency (EIT) in the closed channel to control magnetic Feshbach resonances in an optically-trapped mixture of the two lowest hyperfine states of a 6 Li Fermi gas. In our experiments, the narrow Feshbach resonance is tuned by up to 3 G. For the broad resonance, the spontaneous lifetime is increased to 0.4 s at the dark state resonance, compared to 0.5 ms for single field tuning. We present a new model of light-induced loss spectra, employing continuum-dressed basis states, that agrees in shape and magnitude with loss measurements for both broad and narrow resonances. Using this model, we predict the trade-off between tunability and loss for the broad resonance in 6 Li, showing that our two-field method substantially reduces the two-body loss rate compared to single field methods for same tuning range. This research is supported by AFOSR, NSF, ARO, and DOE.

  9. MEMS tunable optical filter based on multi-ring resonator

    SciTech Connect

    Dessalegn, Hailu E-mail: tsrinu@ece.iisc.ernet.in; Srinivas, T. E-mail: tsrinu@ece.iisc.ernet.in

    2014-10-15

    We propose a novel MEMS tunable optical filter with a flat-top pass band based on multi-ring resonator in an electrostatically actuated microcantilever for communication application. The filter is basically structured on a microcantilever beam and built in optical integrated ring resonator which is placed in one end of the beam to gain maximum stress on the resonator. Thus, when a DC voltage is applied, the beam will bend, that induces a stress and strain in the ring, which brings a change in refractive index and perimeter of the rings leading to change in the output spectrum shift, providing the tenability as high as 0.68nm/μN and it is capable of tuning up to 1.7nm.

  10. Liquid-core optical ring-resonator sensors

    NASA Astrophysics Data System (ADS)

    White, Ian M.; Oveys, Hesam; Fan, Xudong

    2006-05-01

    We have demonstrated a novel sensor architecture based on a liquid-core optical ring-resonator (LCORR) in which a fused silica capillary is utilized to carry the aqueous sample and to act as the ring resonator. The wall thickness of the LCORR is controlled to a few micrometers to expose the whispering gallery mode to the aqueous core. Optical characterization with a water-ethanol mixture shows that the spectral sensitivity of the LCORR sensor is approximately 2.6nm per refractive index unit. A model based on Mie theory is established to explain the experimental results. The LCORR takes advantage of the high sensitivity, small footprint, and low sample consumption with the ring resonator, as well as the efficient fluidic sample delivery with the capillary, and will open an avenue to future multiplexed sensor array development.

  11. Controlling condensate collapse and expansion with an optical Feshbach resonance.

    PubMed

    Yan, Mi; DeSalvo, B J; Ramachandhran, B; Pu, H; Killian, T C

    2013-03-22

    We demonstrate control of the collapse and expansion of an (88)Sr Bose-Einstein condensate using an optical Feshbach resonance near the (1)S(0)-(3)P(1) intercombination transition at 689 nm. Significant changes in dynamics are caused by modifications of scattering length by up to ± 10a(bg), where the background scattering length of (88)Sr is a(bg) = -2a(0) (1a(0) = 0.053 nm). Changes in scattering length are monitored through changes in the size of the condensate after a time-of-flight measurement. Because the background scattering length is close to zero, blue detuning of the optical Feshbach resonance laser with respect to a photoassociative resonance leads to increased interaction energy and a faster condensate expansion, whereas red detuning triggers a collapse of the condensate. The results are modeled with the time-dependent nonlinear Gross-Pitaevskii equation. PMID:25166803

  12. Optical pumping in solid state nuclear magnetic resonance

    SciTech Connect

    Tycko, R.; Reimer, J.A.

    1996-08-01

    An important current trend in solid state nuclear magnetic resonance (NMR) is the growing exploitation of optical pumping of nuclear spin polarizations as a means of enhancing and localizing NMR signals. Recent work has been concentrated in two areas, namely optically pumped NMR in semiconductors and optical pumping of noble gases. Progress in these two areas, including technical developments and new applications in physical chemistry, condensed matter physics, and biomedical sciences, is reviewed. Likely directions for future developments are suggested. 58 refs., 13 figs.

  13. Orbital order of spinless fermions near an optical Feshbach resonance

    SciTech Connect

    Hauke, Philipp; Zhao, Erhai; Goyal, Krittika; Deutsch, Ivan H.; Liu, W. Vincent; Lewenstein, Maciej

    2011-11-15

    We study the quantum phases of a three-color Hubbard model that arises in the dynamics of the p-band orbitals of spinless fermions in an optical lattice. Strong, color-dependent interactions are induced by an optical Feshbach resonance. Starting from the microscopic scattering properties of ultracold atoms, we derive the orbital exchange constants at 1/3 filling on the cubic optical lattice. Using this, we compute the phase diagram in a Gutzwiller ansatz. We find phases with ''axial orbital order'' in which p{sub z} and p{sub x}+ip{sub y} (or p{sub x}-ip{sub y}) orbitals alternate.

  14. Magnetic resonance imaging with an optical atomicmagnetometer

    SciTech Connect

    Xu, Shoujun; Yashchuk, Valeriy V.; Donaldson, Marcus H.; Rochester, Simon M.; Budker, Dmitry; Pines, Alexander

    2006-05-09

    Magnetic resonance imaging (MRI) is a noninvasive andversatile methodology that has been applied in many disciplines1,2. Thedetection sensitivity of conventional Faraday detection of MRI depends onthe strength of the static magnetic field and the sample "fillingfactor." Under circumstances where only low magnetic fields can be used,and for samples with low spin density or filling factor, the conventionaldetection sensitivity is compromised. Alternative detection methods withhigh sensitivity in low magnetic fields are thus required. Here we showthe first use of a laser-based atomic magnetometer for MRI detection inlow fields. Our technique also employs remote detection which physicallyseparates the encoding and detection steps3-5, to improve the fillingfactor of the sample. Potentially inexpensive and using a compactapparatus, our technique provides a novel alternative for MRI detectionwith substantially enhanced sensitivity and time resolution whileavoiding the need for cryogenics.

  15. WGM-Resonator/Tapered-Waveguide White-Light Sensor Optics

    NASA Technical Reports Server (NTRS)

    Stekalov, Dmitry; Maleki, Lute; Matsko, Andrey; Savchenkov, Anatoliy; Iltchenko, Vladimir

    2007-01-01

    Theoretical and experimental investigations have demonstrated the feasibility of compact white-light sensor optics consisting of unitary combinations of (1) low-profile whispering-gallery-mode (WGM) resonators and (2) tapered rod optical waveguides. These sensors are highly wavelength-dispersive and are expected to be especially useful in biochemical applications for measuring absorption spectra of liquids. These sensor optics exploit the properties of a special class of non-diffracting light beams that are denoted Bessel beams because their amplitudes are proportional to Bessel functions of the radii from their central axes. High-order Bessel beams can have large values of angular momentum. In a sensor optic of this type, a low-profile WGM resonator that supports modes having large angular momenta is used to generate high-order Bessel beams. As used here, "low-profile" signifies that the WGM resonator is an integral part of the rod optical waveguide but has a radius slightly different from that of the adjacent part(s).

  16. Supercooling of Atoms in an Optical Resonator

    NASA Astrophysics Data System (ADS)

    Xu, Minghui; Jäger, Simon B.; Schütz, S.; Cooper, J.; Morigi, Giovanna; Holland, M. J.

    2016-04-01

    We investigate laser cooling of an ensemble of atoms in an optical cavity. We demonstrate that when atomic dipoles are synchronized in the regime of steady-state superradiance, the motion of the atoms may be subject to a giant frictional force leading to potentially very low temperatures. The ultimate temperature limits are determined by a modified atomic linewidth, which can be orders of magnitude smaller than the cavity linewidth. The cooling rate is enhanced by the superradiant emission into the cavity mode allowing reasonable cooling rates even for dipolar transitions with ultranarrow linewidth.

  17. Supercooling of Atoms in an Optical Resonator.

    PubMed

    Xu, Minghui; Jäger, Simon B; Schütz, S; Cooper, J; Morigi, Giovanna; Holland, M J

    2016-04-15

    We investigate laser cooling of an ensemble of atoms in an optical cavity. We demonstrate that when atomic dipoles are synchronized in the regime of steady-state superradiance, the motion of the atoms may be subject to a giant frictional force leading to potentially very low temperatures. The ultimate temperature limits are determined by a modified atomic linewidth, which can be orders of magnitude smaller than the cavity linewidth. The cooling rate is enhanced by the superradiant emission into the cavity mode allowing reasonable cooling rates even for dipolar transitions with ultranarrow linewidth. PMID:27127966

  18. High Efficiency Four-Wave Mixing with Relaxation Coupling of Longitude-Optical Phonons in Semiconductor Quantum Wells

    NASA Astrophysics Data System (ADS)

    She, Yan-Chao; Zheng, Xue-Jun; Wang, Deng-Long; Ding, Jian-Wen

    2015-05-01

    The time-dependent analysis of four-wave mixing (FWM) has been performed in four-level double semiconductor quantum wells (SQWs) considering the cross-coupling of the longitude-optical phonons (LOP) relaxation. It is shown that both the amplitude and the conversion efficiency of the FWM field enhance greatly with the increasing strength of cross-coupling of LOP relaxation. Interestingly, a double peak value of the conversion efficiency is obtained under a relatively weak single-photon detuning considering the LOP coupling. When the detuning becomes stronger, the double peaks turn into one peak appearing at the line respect to the about equality two control fields. The results can be interpreted by the effect of electromagnetically induced transparency and the indirect transition. Such controlled high efficiency FWM based on the cross-coupling LOP may have potential applications in quantum control and communications. Supported by Program for Changjiang Scholars and Innovative Research Team in University under Grant (IRT1080), National Natural Science Foundation of China under Grant Nos. 51272158, 11374252, and 51372214, Changjiang Scholar Incentive Program under Grant No. [2009] 17, Scientific Research Fund of Hunan Provincial Education Department of China under Grant No. 12A140, the Science and Technology Foundation of Guizhou Province of China under Grant No. J20122314

  19. Optical coherence tomography with plasmon resonant nanorods of gold

    NASA Astrophysics Data System (ADS)

    Troutman, Timothy S.; Barton, Jennifer K.; Romanowski, Marek

    2007-06-01

    We explored plasmon resonant nanorods of gold as a contrast agent for optical coherence tomography (OCT). Nanorod suspensions were generated through wet chemical synthesis and characterized with spectrophotometry, transmission electron microscopy, and OCT. Polyacrylamide-based phantoms were generated with appropriate scattering and anisotropy coefficients (30 cm-1 and 0.89, respectively) to image distribution of the contrast agent in an environment similar to that of tissue. The observed signal was dependent on whether the plasmon resonance peak overlapped the source bandwidth of the OCT, confirming the resonant character of enhancement. Gold nanorods with plasmon resonance wavelengths overlapping the OCT source yielded a signal-to-background ratio of 4.5 dB, relative to the tissue phantom. Strategies for OCT imaging with nanorods are discussed.

  20. Optical coherence tomography with plasmon resonant nanorods of gold.

    PubMed

    Troutman, Timothy S; Barton, Jennifer K; Romanowski, Marek

    2007-06-01

    We explored plasmon resonant nanorods of gold as a contrast agent for optical coherence tomography (OCT). Nanorod suspensions were generated through wet chemical synthesis and characterized with spectrophotometry, transmission electron microscopy, and OCT. Polyacrylamide-based phantoms were generated with appropriate scattering and anisotropy coefficients (30 cm(-1) and 0.89, respectively) to image distribution of the contrast agent in an environment similar to that of tissue. The observed signal was dependent on whether the plasmon resonance peak overlapped the source bandwidth of the OCT, confirming the resonant character of enhancement. Gold nanorods with plasmon resonance wavelengths overlapping the OCT source yielded a signal-to-background ratio of 4.5 dB, relative to the tissue phantom. Strategies for OCT imaging with nanorods are discussed. PMID:17546147

  1. High sensitivity optical waveguide accelerometer based on Fano resonance.

    PubMed

    Wan, Fenghua; Qian, Guang; Li, Ruozhou; Tang, Jie; Zhang, Tong

    2016-08-20

    An optical waveguide accelerometer based on tunable asymmetrical Fano resonance in a ring-resonator-coupled Mach-Zehnder interferometer (MZI) is proposed and analyzed. A Fano resonance accelerometer has a relatively large workspace of coupling coefficients with high sensitivity, which has potential application in inertial navigation, missile guidance, and attitude control of satellites. Due to the interference between a high-Q resonance pathway and a coherent background pathway, a steep asymmetric line shape is generated, which greatly improves the sensitivity of this accelerometer. The sensitivity of the accelerometer is about 111.75 mW/g. A 393-fold increase in sensitivity is achieved compared with a conventional MZI accelerometer and is approximately equal to the single ring structure. PMID:27556984

  2. Synchronization of optically coupled resonant tunneling diode oscillators

    NASA Astrophysics Data System (ADS)

    Romeira, Bruno; Figueiredo, José M. L.; Ironside, Charles N.; Quintana, José M.

    2013-11-01

    We experimentally investigate the synchronous response of two fiber-optic coupled optoelectronic circuit oscillators based on resonant tunneling diodes (RTDs). The fiber-optic synchronization link employs injection of a periodic oscillating optical modulated signal generated by a master RTD-laser diode (LD) oscillator to a slave RTD-photodetector (PD) oscillator. The synchronous regimes were evaluated as a function of frequency detuning and optical injection strength. The results show the slave RTD-PD oscillator follows the frequency and noise characteristics of the master RTD-LD oscillator resulting in two oscillators with similar phase noise characteristics exhibiting single side band phase noise levels below -100 dBc/Hz at 1 MHz offset from the carrier frequency. Optical synchronization of RTD-based optoelectronic circuit oscillators have many applications spanning from sensing, to microwave generation, and data transmission.

  3. A phononic crystal strip based on silicon for support tether applications in silicon-based MEMS resonators and effects of temperature and dopant on its band gap characteristics

    NASA Astrophysics Data System (ADS)

    Ha, Thi Dep; Bao, JingFu

    2016-04-01

    Phononic crystals (PnCs) and n-type doped silicon technique have been widely employed in silicon-based MEMS resonators to obtain high quality factor (Q) as well as temperature-induced frequency stability. For the PnCs, their band gaps play an important role in the acoustic wave propagation. Also, the temperature and dopant doped into silicon can cause the change in its material properties such as elastic constants, Young's modulus. Therefore, in order to design the simultaneous high Q and frequency stability silicon-based MEMS resonators by two these techniques, a careful design should study effects of temperature and dopant on the band gap characteristics to examine the acoustic wave propagation in the PnC. Based on these, this paper presents (1) a proposed silicon-based PnC strip structure for support tether applications in low frequency silicon-based MEMS resonators, (2) influences of temperature and dopant on band gap characteristics of the PnC strips. The simulation results show that the largest band gap can achieve up to 33.56 at 57.59 MHz and increase 1280.13 % (also increase 131.89 % for ratio of the widest gaps) compared with the counterpart without hole. The band gap properties of the PnC strips is insignificantly effected by temperature and electron doping concentration. Also, the quality factor of two designed length extensional mode MEMS resonators with proposed PnC strip based support tethers is up to 1084.59% and 43846.36% over the same resonators with PnC strip without hole and circled corners, respectively. This theoretical study uses the finite element analysis in COMSOL Multiphysics and MATLAB softwares as simulation tools. This findings provides a background in combination of PnC and dopant techniques for high performance silicon-based MEMS resonators as well as PnC-based MEMS devices.

  4. Optical micro-bubble resonators as promising biosensors

    NASA Astrophysics Data System (ADS)

    Giannetti, A.; Barucci, A.; Berneschi, S.; Cosci, A.; Cosi, F.; Farnesi, D.; Nunzi Conti, G.; Pelli, S.; Soria, S.; Tombelli, S.; Trono, C.; Righini, G. C.; Baldini, F.

    2015-05-01

    Recently, optical micro-bubble resonators (OMBRs) have gained an increasing interest in many fields of photonics thanks to their particular properties. These hollow microstructures can be suitable for the realization of label - free optical biosensors by combining the whispering gallery mode (WGM) resonator properties with the intrinsic capability of integrated microfluidics. In fact, the WGMs are morphology-dependent modes: any change on the OMBR inner surface (due to chemical and/or biochemical binding) causes a shift of the resonance position and reduces the Q factor value of the cavity. By measuring this shift, it is possible to obtain information on the concentration of the analyte to be detected. A crucial step for the development of an OMBR-based biosensor is constituted by the functionalization of its inner surface. In this work we report on the development of a physical and chemical process able to guarantee a good homogeneity of the deposed bio-layer and, contemporary, to preserve a high quality factor Q of the cavity. The OMBR capability of working as bioassay was proved by different optical techniques, such as the real time measurement of the resonance broadening after each functionalization step and fluorescence microscopy.

  5. Optical distributed sensors for feedback control: Characterization of photorefractive resonator

    NASA Technical Reports Server (NTRS)

    Indebetouw, Guy; Lindner, D. K.

    1992-01-01

    The aim of the project was to explore, define, and assess the possibilities of optical distributed sensing for feedback control. This type of sensor, which may have some impacts in the dynamic control of deformable structures and the monitoring of small displacements, can be divided into data acquisition, data processing, and control design. Analogue optical techniques, because they are noninvasive and afford massive parallelism may play a significant role in the acquisition and the preprocessing of the data for such a sensor. Assessing these possibilities was the aim of the first stage of this project. The scope of the proposed research was limited to: (1) the characterization of photorefractive resonators and the assessment of their possible use as a distributed optical processing element; and (2) the design of a control system utilizing signals from distributed sensors. The results include a numerical and experimental study of the resonator below threshold, an experimental study of the effect of the resonator's transverse confinement on its dynamics above threshold, a numerical study of the resonator above threshold using a modal expansion approach, and the experimental test of this model. A detailed account of each investigation, including methodology and analysis of the results are also included along with reprints of published and submitted papers.

  6. Resonant modes of optical cavities with phase-conjugate mirrors.

    PubMed

    Bélanger, P A; Hardy, A; Siegman, A E

    1980-02-15

    The lowest-order self-consistent Gaussian transverse modes are derived, also the resonant frequencies of an optical resonator formed by conventional paraxial optical components plus a phase-conjugate mirror (PCM) on one end. The conventional optical elements are described by an over-all ABCD matrix. Cavities with purely real elements (no aperturing) have a continuous set of self-reproducing Gaussian modes described by a semicircular locus in the 1/q plane for one round trip; all Gaussian beams are self-reproducing after two round trips. Complex ABCD matrices, such as are produced by Gaussian aperturing in the cavity, lead to unique self-consistent perturbation-stable Gaussian modes. The resonant frequency spectrum of a PCM cavity consists of a central resonance at the driving frequency omega(0) of the PCM element, independent of the cavity length L, plus half-axial sidebands spaced by Deltaomega(ax) = 2pi(c/4L), with phase and amplitude constraints on each pair of upper and lower sidebands. PMID:20216900

  7. Optically confined polarized resonance Raman studies in identifying crystalline orientation of sub-diffraction limited AlGaN nanostructure

    SciTech Connect

    Sivadasan, A. K. Patsha, Avinash; Dhara, Sandip

    2015-04-27

    An optical characterization tool of Raman spectroscopy with extremely weak scattering cross section tool is not popular to analyze scattered signal from a single nanostructure in the sub-diffraction regime. In this regard, plasmonic assisted characterization tools are only relevant in spectroscopic studies of nanoscale object in the sub-diffraction limit. We have reported polarized resonance Raman spectroscopic (RRS) studies with strong electron-phonon coupling to understand the crystalline orientation of a single AlGaN nanowire of diameter ∼100 nm. AlGaN nanowire is grown by chemical vapor deposition technique using the catalyst assisted vapor-liquid-solid process. The results are compared with the high resolution transmission electron microscopic analysis. As a matter of fact, optical confinement effect due to the dielectric contrast of nanowire with respect to that of surrounding media assisted with electron-phonon coupling of RRS is useful for the spectroscopic analysis in the sub-diffraction limit of 325 nm (λ/2N.A.) using an excitation wavelength (λ) of 325 nm and near ultraviolet 40× far field objective with a numerical aperture (N.A.) value of 0.50.

  8. Phonon-mediated magnetic polaritons
in the infrared region.

    PubMed

    Wang, L P; Zhang, Z M

    2011-03-14

    Magnetic polaritons that couple electromagnetic waves with magnetic excitation can be used for tailoring the radiative properties of materials in energy-harvesting and other applications. Previous studies used metallic microstructures to induce magnetic responses. With rigorous coupled-wave analysis (RCWA), transmission enhancement with a SiC slit array and coherent thermal emission with a SiC deep grating is theoretically demonstrated in the infrared within the phonon absorption band. The field distributions and the agreement in the resonance frequencies predicted from both RCWA and LC circuit models strongly suggest that magnetic polaritons exist in the SiC microstructures. This type of magnetic polariton is mediated by vibration of atoms in polar materials (i.e., optical phonons), rather than by free electrons in metals. Our results suggest that phonon-mediated magnetic polaritons have promising applications such as filters and selective coherent emitters in the infrared spectral region. PMID:21445214

  9. Miscibility gap and phonon thermodynamics of Fe-Au alloys studied by inelastic neutron scattering and nuclear-resonant inelastic x-ray scattering

    SciTech Connect

    Muñoz, Jorge A.; Fultz, Brent

    2015-07-23

    Recent measurements of the phonon spectra of several Au-rich alloys of face-centered-cubic Fe-Au using inelastic neutron scattering and nuclear-resonant inelastic x-ray scattering are summarized. The Wills-Harrison model, accounting for charge transfer upon alloying, is used to explain the observed negative excess vibrational entropy of mixing, which increases the miscibility gap temperature in the system by an estimated maximum of 550 K and we adjudicate to a charge transfer from the Fe to the Au atoms that results in an increase in the electron density in the free-electron-like states and in stronger sd-hybridization. When Au is the solvent, this softens the Fe–Fe bonds but stiffens the Au–Au and Au–Fe bonds which results in a net stiffening relative to the elemental components.

  10. Optical resonant ultrasound spectroscopy for spherical target characterization

    SciTech Connect

    Hale, Tom

    2010-01-01

    A new non-contact resonant ultrasound spectroscopic technique is employed to determine the response characteristics of spherical fusion targets, with particular emphasis on both the displacement sensitivity and frequency response of the technique. The optical experimental method is based on photorefractive optical lock-in detection scheme with narrow bandwidth amplification to measure phase variations in light scattered from optically rough, continuously vibrating surfaces with very high, linear sensitivity and a noise level on the order of 10.6 nanometers RMS. This high sensitivity is needed to determine the vibrational modes of the gas inside an spherical target separately from the elastic modes of the containment shell. These measurements can be used to calculate the pressure and density of the internal gas. This approach is also used to discriminate between nearly-degenerate resonant modes characteristic of the frequency spectrum when the target fabrication is inadequate (non-uniform shell thickness, misalignment of hemispheres) or when the Deuteriumrrritium solid fuel inside the target is not symmetrically distributed at cryogenic temperatures. Asymmetries in the fuel layering and geometric perturbations disturb the target implosion process creating deleterious effects in fusion energy generation. The technique is applied to determine the modal characteristics of a target sphere with known response from 100 KHz to 450 KHz. The results demonstrate the unique capabilities of the optical lock-in detection method to measure very small resonant ultrasonic signals.

  11. Manipulation of resonant Auger processes with strong optical fields

    NASA Astrophysics Data System (ADS)

    Picón, Antonio; Buth, Christian; Doumy, Gilles; Krässig, Bertold; Young, Linda; Southworth, Stephen

    2013-05-01

    We recently reported on the optical control of core-excited states of a resonant Auger process in neon. We have focused on the resonant excitation 1 s --> 1s-1 3 p , while a strong optical field may resonantly couple two core-excited states (1s-1 3 p and 1s-1 3 s) in the Rydberg manifold as well as dressing the continuum. There is a clear signature in the Auger electron spectrum of the inner-shell dynamics induced by the strong optical field: i) the Auger electron spectrum is modified by the rapid optical-induced population transfer from the 1s-1 3 p state to the 1s-1 3 s state during their decay. ii) The angular anisotropy parameter, defining the angular distribution of the Auger electron, is manifested in the envelope of the (angle-integrated) sidebands. This work is funded by the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy, under Contract No. DE-AC02-06CH11357.

  12. A fiber-optic hydrophone with a cylindrical Helmholtz resonator

    NASA Astrophysics Data System (ADS)

    Wang, Zefeng; Hu, Yongming; Ni, Ming; Meng, Zhou; Luo, Hong

    2007-11-01

    A passive homodyne Michelson interferometric fiber-optic hydrophone with a single-hole cylindrical Helmholtz resonator has been manufactured. To validate the theoretical results that the fluid coefficient of viscosity has great influence on the maximum sensitivity at the resonant frequency, the acoustic sensitivity frequency response of the fiber-optic hydrophone has been measured in a standing-wave tank filled with castor oil. The viscosity coefficient of castor oil will change with the variation of the temperature. Experimental Results show that the fiber-optic hydrophone frequency responses of different temperature have identical form except that the maximum sensitivities are different. The acoustic sensitivities of low frequency are about -159dB re 1rad/μPa. While the maximum sensitivities near the measured resonant frequency of 800Hz go down with the fall of the temperature, i.e. with the increase of the viscosity coefficient, which is agree with the theoretical conclusions. This fiber-optic hydrophone is a prototype device for a class of sensors that used to eliminate aliasing in the future sonar systems.

  13. Bistable moving optical solitons in resonant photonic crystals

    SciTech Connect

    Vlasov, R. A.; Lemeza, A. M.

    2011-08-15

    We consider some new aspects of the formation of moving optical solitons in a medium of Bragg-type resonant grating doped with two-level atoms. For generality, account is taken of the local-field effect assisted by a sufficiently high density of resonant atoms. It is established analytically that there exists a family of soliton solutions to the two-wave Maxwell-Bloch system of equations, with these solitons exhibiting bistable properties. The existence of bistable solitons and their properties are confirmed by numerical simulations.

  14. Effect of the direct capture of holes with the emission of optical phonons on impurity-photoconductivity relaxation in p-Si:B

    SciTech Connect

    Kozlov, D. V. Morozov, S. V.; Rumyantsev, V. V.; Tuzov, I. V.; Kudryavtsev, K. E.; Gavrilenko, V. I.

    2015-02-15

    A theoretical model developed for interpretation of the results of measurements of the impurity-photoconductivity relaxation in p-Si:B under pulsed optical excitation by a narrow-band tunable source of radiation in “heating” (10–500 V/cm) electric fields is presented. The model takes into account the capture of holes at the ground and lower excited states of boron with optical-phonon emission. It is shown that the dependence of the photoconductivity-relaxation time on the electric-field intensity can be unsteady taking into account these processes.

  15. Single spin optically detected magnetic resonance with 60-90 GHz (E-band) microwave resonators.

    PubMed

    Aslam, Nabeel; Pfender, Matthias; Stöhr, Rainer; Neumann, Philipp; Scheffler, Marc; Sumiya, Hitoshi; Abe, Hiroshi; Onoda, Shinobu; Ohshima, Takeshi; Isoya, Junichi; Wrachtrup, Jörg

    2015-06-01

    Magnetic resonance with ensembles of electron spins is commonly performed around 10 GHz, but also at frequencies above 240 GHz and in corresponding magnetic fields of over 9 T. However, experiments with single electron and nuclear spins so far only reach into frequency ranges of several 10 GHz, where existing coplanar waveguide structures for microwave (MW) delivery are compatible with single spin readout techniques (e.g., electrical or optical readout). Here, we explore the frequency range up to 90 GHz, with magnetic fields of up to ≈3 T for single spin magnetic resonance in conjunction with optical spin readout. To this end, we develop MW resonators with optical single spin access. In our case, rectangular 60-90 GHz (E-band) waveguides guarantee low-loss supply of microwaves to the resonators. Three dimensional cavities, as well as coplanar waveguide resonators, enhance MW fields by spatial and spectral confinement with a MW efficiency of 1.36 mT/√W. We utilize single nitrogen vacancy (NV) centers as hosts for optically accessible spins and show that their properties regarding optical spin readout known from smaller fields (<0.65 T) are retained up to fields of 3 T. In addition, we demonstrate coherent control of single nuclear spins under these conditions. Furthermore, our results extend the applicable magnetic field range of a single spin magnetic field sensor. Regarding spin based quantum registers, high fields lead to a purer product basis of electron and nuclear spins, which promises improved spin lifetimes. For example, during continuous single-shot readout, the (14)N nuclear spin shows second-long longitudinal relaxation times. PMID:26133855

  16. Optics and biophotonics of nanoparticles with a plasmon resonance

    SciTech Connect

    Khlebtsov, N G

    2008-06-30

    A brief review of the state of the art in theoretical and experimental studies of the optical properties of metal particles with dipole and multipole plasmon resonances is presented. Metal spheres, nanorods, spherical and elliptic metal nanoshells are considered. The tuning of plasmon resonances of nanoparticles by varying their size, shape, structure, and dielectric environment is described. A large amount of spectrophotometric data on dimensional characteristics of gold colloidal particles is critically analysed and a new calibration of the dependence of their average size on the extinction plasmon resonance wavelength is proposed. A drastic difference between gold and silver colloids in the region of small deviations of their form from spherical is discussed. An example of the excess over not only the Rayleigh limit for the scattering depolarisation factor for dielectric needles (1/3) but also over the plasmon-resonance limit for metal thin rods (3/4) is presented for the first time. The multipole properties of nanorods and universal linear wavelength scaling of multipole resonances are considered depending on the axial ratio of nanoparticles. The outlook for modern trends in biomedical applications of nanoparticles with plasmon resonances is discussed. (special issue devoted to application of laser technologies in biophotonics and biomedical studies)

  17. Enhanced Light Scattering of the Forbidden longitudinal Optical Phonon Mode Studied by Micro-Raman Spectroscopy on Single InN nanowires

    SciTech Connect

    Sutter, E.; Schafer-Nolte, E.O.; Stoica T.; Gotschke, T.; Limbach, F.A.; Sutter, P.; Grutzmacher, D.; Calarco, R.

    2010-08-06

    In the literature, there are controversies on the interpretation of the appearance in InN Raman spectra of a strong scattering peak in the energy region of the unscreened longitudinal optical (LO) phonons, although a shift caused by the phonon-plasmon interaction is expected for the high conductance observed in this material. Most measurements on light scattering are performed on ensembles of InN nanowires (NWs). However, it is important to investigate the behavior of individual nanowires and here we report on micro-Raman measurements on single nanowires. When changing the polarization direction of the incident light from parallel to perpendicular to the wire, the expected reduction of the Raman scattering was observed for transversal optical (TO) and E2 phonon scattering modes, while a strong symmetry-forbidden LO mode was observed independently on the laser polarization direction. Single Mg- and Si-doped crystalline InN nanowires were also investigated. Magnesium doping results in a sharpening of the Raman peaks, while silicon doping leads to an asymmetric broadening of the LO peak. The results can be explained based on the influence of the high electron concentration with a strong contribution of the surface accumulation layer and the associated internal electric field.

  18. Electron-phonon processes of the nitrogen-vacancy center in diamond

    NASA Astrophysics Data System (ADS)

    Plakhotnik, Taras; Doherty, Marcus W.; Manson, Neil B.

    2015-08-01

    Applications of the negatively charged nitrogen-vacancy center in diamond exploit the center's unique optical and spin properties, which at ambient temperature are predominately governed by electron-phonon interactions. Here, we investigate these interactions at ambient and elevated temperatures by observing the motional narrowing of the center's excited-state spin resonances. We determine that the center's Jahn-Teller dynamics are much slower than currently believed and that they do not solely account for the broadening of the center's optical resonance above cryogenic temperatures. We show that the inclusion of interactions with symmetric phonon modes can explain the observed broadening and resolve the current inconsistencies in the literature. However, our model also reveals unexpected features of the electron-phonon processes that coincide with other poorly understood vibronic features of the center and require further investigation.

  19. Surface plasmon resonance based fiber optic glucose biosensor

    NASA Astrophysics Data System (ADS)

    Srivastava, Sachin K.; Verma, Roli; Gupta, Banshi D.

    2012-02-01

    A surface plasmon resonance (SPR) based fiber optic biosensor has been fabricated and characterized for the detection of blood glucose. Optical fiber sensor was fabricated by first coating a 50 nm thick gold film on the bare core of optical fiber and then immobilizing glucose oxidase (GOx) over it. Aqueous glucose solutions of different concentrations were prepared. To mimic the blood glucose levels, the concentration of glucose solutions were kept equal to that in human blood. The refractive indices of these sample solutions were equal to that of water up to third decimal place. SPR spectra for the sensor were recorded for these glucose solutions. When the glucose comes in contact to glucose oxidase, chemical reactions take place and as a result, the refractive index of the immobilized GOx film changes, giving rise to a shift in the resonance wavelength. Unlike electrochemical sensors, the present sensor is based on optics and can be miniaturized because of optical fiber. The present study provides a different approach for blood glucose sensing and may be commercialized after optimization of certain parameters.

  20. The ``Music'' of Light: Optical Resonances for Fun and Profit

    NASA Astrophysics Data System (ADS)

    Beausoleil, Raymond

    Moore's Law has set great expectations that the performance/price ratio of commercially available semiconductor devices will continue to improve exponentially at least until the end of this decade. But the physics of the metal wires that connect the transistors on a silicon chip already places stringent limits on the performance of integrated circuits, making their continued dramatic improvement highly unlikely. In this talk, I will introduce the basic concept of an optical resonance in a microscopic dielectric cavity in the context of the same type of spatial boundary conditions that give each musical instrument its unique sound. Then I will illustrate applications of these resonances to information technology in a variety of forms and functions using examples from my own laboratory at HP, such as chip-scale optical networks, quantum bits based on spins in diamond, and ultrafast optical switches that could become the foundation for a new generation of optical computers. Our goal is to conduct advanced research that could precipitate an ``optical Moore's Law'' and allow exponential performance gains to continue through the end of the next decade.

  1. Magneto-optical switching devices based on Si resonators

    NASA Astrophysics Data System (ADS)

    Noda, Kazuki; Okada, Kazuya; Amemiya, Yoshiteru; Yokoyama, Shin

    2016-04-01

    The magneto-optical switching devices based on Si ring and Si photonic crystal resonators have been fabricated using a Bi3Fe5O12 (BIG) film deposited by the metal organic decomposition (MOD) method. The quality of the obtained BIG film was evaluated by X-ray diffraction and the magneto-optical Kerr effect and relatively good results were obtained. The light modulations of both devices were ≦20% at a wavelength of ˜1.5 µm. The operation mechanisms of both devices are explained by the Cotton-Mouton effect where the magnetic field direction is perpendicular to the light propagation direction.

  2. Label-free optical resonant sensors for biochemical applications

    NASA Astrophysics Data System (ADS)

    Ciminelli, Caterina; Campanella, Clarissa Martina; Dell'Olio, Francesco; Campanella, Carlo Edoardo; Armenise, Mario Nicola

    2013-03-01

    For a number of years, the scientific community has been paying growing attention to the monitoring and enhancement of public health and the quality of life through the detection of all dangerous agents for the human body, including gases, proteins, virus, and bacterial agents. When these agents are detected through label-free biochemical sensors, the molecules are not modified structurally or functionally by adding fluorescent or radioactive dyes. This work focuses on label-free optical ring resonator-based configurations suited for bio-chemical sensing, highlighting their physical aspects and specific applications. Resonant wavelength shift and the modal splitting occurring when the analyte interacts with microresonant structures are the two major physical aspects analyzed in this paper. Competitive optical platforms proposed in the literature are also illustrated together with their properties and performance.

  3. Feedback-free optical cavity with self-resonating mechanism

    NASA Astrophysics Data System (ADS)

    Uesugi, Y.; Hosaka, Y.; Honda, Y.; Kosuge, A.; Sakaue, K.; Omori, T.; Takahashi, T.; Urakawa, J.; Washio, M.

    2016-05-01

    We demonstrated the operation of a high finesse optical cavity without utilizing an active feedback system to stabilize the resonance. The effective finesse, which is a finesse including the overall system performance, of the cavity was measured to be 394 000 ± 10 000, and the laser power stored in the cavity was 2.52 ± 0.13 kW, which is approximately 187 000 times greater than the incident power to the cavity. The stored power was stabilized with a fluctuation of 1.7%, and we confirmed continuous cavity operation for more than two hours. This result has the potential to trigger an innovative evolution for applications that use optical resonant cavities such as compact photon sources with laser-Compton scattering or cavity enhanced absorption spectroscopy.

  4. Research progress of the resonant fiber optic gyroscope technology

    NASA Astrophysics Data System (ADS)

    Wang, Linglan; Yan, Yuchao; Ma, Huilian; Jin, Zhonghe

    2015-10-01

    The resonant fiber optic gyro (RFOG) is a high accuracy inertial rotation sensor based on the Sagnac effect. The existence of various noises, including the nonreciprocal noises such as the polarization noise and the Kerr noise as well as the reciprocal circuit noise, limits the performance improvement of the RFOG. An improved scheme by inserting two in-line polarizers in the polarization maintaining fiber transmission-type resonator has been proposed to suppress the polarization-fluctuation induced drift. Furthermore, the adoption of the air-core photonic bandgap fibers (PBFs) offers a novel solution to reduce the optical Kerr effect. In addition, A digital signal processor is designed to reduce the reciprocal noises and detect the rotation information. A minimum actual rotation of 0.001°/s is achieved. The dynamic range is improved by a factor of 7 and the scale factor nonlinearity is decreased by a factor of 60.

  5. Capture into resonance and phase space dynamics in optical centrifuge

    NASA Astrophysics Data System (ADS)

    Armon, Tsafrir; Friedland, Lazar

    2016-05-01

    The process of capture of a molecular enesemble into rotational resonance in the optical centrifuge is investigated. The adiabaticity and phase space incompressibility are used to find the resonant capture probability in terms of two dimensionless parameters P1 , 2 characterising the driving strength and the nonlinearity, and related to three characteristic time scales in the problem. The analysis is based on the transformation to action-angle variables and the single resonance approximation, yielding reduction of the three-dimensional rotation problem to one degree of freedom. The analytic results for capture probability are in a good agreement with simulations. The existing experiments satisfy the validity conditions of the theory. This work was supported by the Israel Science Foundation Grant 30/14.

  6. Fano resonance based optical modulator reaching 85% modulation depth

    NASA Astrophysics Data System (ADS)

    Zhao, Wenyu; Jiang, Huan; Liu, Bingyi; Jiang, Yongyuan; Tang, Chengchun; Li, Junjie

    2015-10-01

    In this paper, we demonstrate the combination of nematic liquid crystal with a binary silicon nanohole array to realize a high performance Fano resonance based optical modulator. The simulations using a finite difference time domain method reveal that the sharp Fano profile in the binary array originates from the interaction of the in-phased and anti-phased lattice collective resonance hybridized through lattice coupling effects. Experimental results agree very well with the simulations and demonstrate the strong dependence of the Q factor and spectral contrast of the resonance on the radius difference of the two nanohole arrays. Infiltrated with nematic liquid crystal, E7, the Fano profile can be dynamically and continuously tuned by an applied voltage, and an unprecedented modulation depth up to 85% is achieved.

  7. Active mode-locked lasers and other photonic devices using electro-optic whispering gallery mode resonators

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey B. (Inventor); Ilchenko, Vladimir (Inventor); Savchenkov, Anatoliy (Inventor); Maleki, Lutfollah (Inventor)

    2006-01-01

    Techniques and devices using whispering gallery mode (WGM) optical resonators, where the optical materials of the WGM resonators exhibit an electro-optical effect to perform optical modulation. Examples of actively mode-locked lasers and other devices are described.

  8. Electron paramagnetic resonance and optical absorption spectral studies on chalcocite

    NASA Astrophysics Data System (ADS)

    Reddy, S. Lakshmi; Fayazuddin, Md.; Frost, Ray L.; Endo, Tamio

    2007-11-01

    A chalcocite mineral sample of Shaha, Congo is used in the present study. An electron paramagnetic resonance (EPR) study on powdered sample confirms the presence of Mn(II), Fe(III) and Cu(II). Optical absorption spectrum indicates that Fe(III) impurity is present in octahedral structure whereas Cu(II) is present in rhombically distorted octahedral environment. Mid-infrared results are due to water and sulphate fundamentals.

  9. Electron paramagnetic resonance and optical absorption spectral studies on chalcocite.

    PubMed

    Reddy, S Lakshmi; Fayazuddin, Md; Frost, Ray L; Endo, Tamio

    2007-11-01

    A chalcocite mineral sample of Shaha, Congo is used in the present study. An electron paramagnetic resonance (EPR) study on powdered sample confirms the presence of Mn(II), Fe(III) and Cu(II). Optical absorption spectrum indicates that Fe(III) impurity is present in octahedral structure whereas Cu(II) is present in rhombically distorted octahedral environment. Mid-infrared results are due to water and sulphate fundamentals. PMID:17324611

  10. p-wave optical Feshbach resonances in {sup 171}Yb

    SciTech Connect

    Goyal, Krittika; Deutsch, Ivan; Reichenbach, Iris

    2010-12-15

    We study the use of an optical Feshbach resonance to modify the p-wave interaction between ultracold polarized {sup 171}Yb spin-1/2 fermions. A laser exciting two colliding atoms to the {sup 1}S{sub 0}+{sup 3}P{sub 1} channel can be detuned near a purely-long-range excited molecular bound state. Such an exotic molecule has an inner turning point far from the chemical binding region, and thus, three-body recombination in the Feshbach resonance will be highly suppressed in contrast to that typically seen in a ground-state p-wave magnetic Feshbach resonance. We calculate the excited molecular bound-state spectrum using a multichannel integration of the Schroedinger equation, including an external perturbation by a magnetic field. From the multichannel wave functions, we calculate the Feshbach resonance properties, including the modification of the elastic p-wave scattering volume and inelastic spontaneous scattering rate. The use of magnetic fields and selection rules for polarized light yields a highly controllable system. We apply this control to propose a toy model for three-color superfluidity in an optical lattice for spin-polarized {sup 171}Yb, where the three colors correspond to the three spatial orbitals of the first excited p band. We calculate the conditions under which tunneling and on-site interactions are comparable, at which point quantum critical behavior is possible.

  11. Quasi-transverse optical phonon mode in self-generated semipolar AlN grains embedded in c-oriented AlN matrix grown on sapphire using hydride vapor phase epitaxy

    NASA Astrophysics Data System (ADS)

    Hu, Y. Y.; Zhou, T. F.; Zheng, S. N.; Liu, X. H.; Zhao, J. J.; Su, X. J.; Huang, J.; Qiu, Y. X.; Zhang, J. C.; Xu, K.

    2016-05-01

    In this study, we present a microspectroscopic investigation on the quasi-transverse optical phonon modes Q(TO) in some self-generated aluminum nitride (AlN) grains grown on sapphire using hydride vapor phase epitaxy. Using X-ray diffraction and transmission electron microscope, these grains were confirmed to be embedded in (0001)-AlN (c-AlN) epitaxial matrix with an appearance plane of (10 1 ¯ 1 ) (s-plane). Two beam bright field images further showed that the AlN grains were free of dislocation. In-plane phonon anisotropy of the AlN grains was discussed in detail using angular-dependent polarized Raman spectroscopy. The dependence of pure Raman phonons intensity on rotation angle agrees well with the calculation. The Q(TO) phonon intensity exhibited similar behavior to that of A1(TO) phonon, which can be explained by Loudon's formula. However, the observed frequency fluctuation for the Q(TO) phonon differs from that of the pure phonon modes, which cannot be directly understood from the classic Loudon's formula. A modified Loudon's formula appropriate to non-normal incidence was presented to explain the observed Q(TO) phonon frequency fluctuation. Combining with the angular-dependent Raman spectra, we proposed that a small inclination of s-plane along with the various in-plane orientations in c-AlN matrix lead to the frequency fluctuation of Q(TO) in these embedded semipolar AlN grains.

  12. Resonance Frequency of Optical Microbubble Resonators: Direct Measurements and Mitigation of Fluctuations.

    PubMed

    Cosci, Alessandro; Berneschi, Simone; Giannetti, Ambra; Farnesi, Daniele; Cosi, Franco; Baldini, Francesco; Nunzi Conti, Gualtiero; Soria, Silvia; Barucci, Andrea; Righini, Giancarlo; Pelli, Stefano

    2016-01-01

    This work shows the improvements in the sensing capabilities and precision of an Optical Microbubble Resonator due to the introduction of an encaging poly(methyl methacrylate) (PMMA) box. A frequency fluctuation parameter σ was defined as a score of resonance stability and was evaluated in the presence and absence of the encaging system and in the case of air- or water-filling of the cavity. Furthermore, the noise interference introduced by the peristaltic and the syringe pumping system was studied. The measurements showed a reduction of σ in the presence of the encaging PMMA box and when the syringe pump was used as flowing system. PMID:27589761

  13. Depth dependent modification of optical constants arising from H+ implantation in n-type 4H-SiC measured using coherent acoustic phonons

    NASA Astrophysics Data System (ADS)

    Baydin, Andrey; Krzyzanowska, Halina; Dhanunjaya, Munthala; Nageswara Rao, S. V. S.; Davidson, Jimmy L.; Feldman, Leonard C.; Tolk, Norman H.

    2016-06-01

    Silicon carbide (SiC) is a promising material for new generation electronics including high power/high temperature devices and advanced optical applications such as room temperature spintronics and quantum computing. Both types of applications require the control of defects particularly those created by ion bombardment. In this work, modification of optical constants of 4H-SiC due to hydrogen implantation at 180 keV and at fluences ranging from 1014 to 1016 cm-2 is reported. The depth dependence of the modified optical constants was extracted from coherent acoustic phonon spectra. Implanted spectra show a strong dependence of the 4H-SiC complex refractive index depth profile on H+ fluence. These studies provide basic insight into the dependence of optical properties of 4H silicon carbide on defect densities created by ion implantation, which is of relevance to the fabrication of SiC-based photonic and optoelectronic devices.

  14. Phononic plate waves.

    PubMed

    Wu, Tsung-Tsong; Hsu, Jin-Chen; Sun, Jia-Hong

    2011-10-01

    In the past two decades, phononic crystals (PCs) which consist of periodically arranged media have attracted considerable interest because of the existence of complete frequency band gaps and maneuverable band structures. Recently, Lamb waves in thin plates with PC structures have started to receive increasing attention for their potential applications in filters, resonators, and waveguides. This paper presents a review of recent works related to phononic plate waves which have recently been published by the authors and coworkers. Theoretical and experimental studies of Lamb waves in 2-D PC plate structures are covered. On the theoretical side, analyses of Lamb waves in 2-D PC plates using the plane wave expansion (PWE) method, finite-difference time-domain (FDTD) method, and finite-element (FE) method are addressed. These methods were applied to study the complete band gaps of Lamb waves, characteristics of the propagating and localized wave modes, and behavior of anomalous refraction, called negative refraction, in the PC plates. The theoretical analyses demonstrated the effects of PC-based negative refraction, lens, waveguides, and resonant cavities. We also discuss the influences of geometrical parameters on the guiding and resonance efficiency and on the frequencies of waveguide and cavity modes. On the experimental side, the design and fabrication of a silicon-based Lamb wave resonator which utilizes PC plates as reflective gratings to form the resonant cavity are discussed. The measured results showed significant improvement of the insertion losses and quality factors of the resonators when the PCs were applied. PMID:21989878

  15. Coherent acoustic phonons in nanostructures

    NASA Astrophysics Data System (ADS)

    Dekorsy, T.; Taubert, R.; Hudert, F.; Bartels, A.; Habenicht, A.; Merkt, F.; Leiderer, P.; Köhler, K.; Schmitz, J.; Wagner, J.

    2008-02-01

    Phonons are considered as a most important origin of scattering and dissipation for electronic coherence in nanostructures. The generation of coherent acoustic phonons with femtosecond laser pulses opens the possibility to control phonon dynamics in amplitude and phase. We demonstrate a new experimental technique based on two synchronized femtosecond lasers with GHz repetition rate to study the dynamics of coherently generated acoustic phonons in semiconductor heterostructures with high sensitivity. High-speed synchronous optical sampling (ASOPS) enables to scan a time-delay of 1 ns with 100 fs time resolution with a frequency in the kHz range without a moving part in the set-up. We investigate the dynamics of coherent zone-folded acoustic phonons in semiconductor superlattices (GaAs/AlAs and GaSb/InAs) and of coherent vibration of metallic nanostructures of non-spherical shape using ASOPS.

  16. Direct electrical-to-optical conversion and light modulation in micro whispering-gallery-mode resonators

    NASA Technical Reports Server (NTRS)

    Maleki, Lute (Inventor); Levi, Anthony F. J. (Inventor)

    2005-01-01

    Techniques for directly converting an electrical signal into an optical signal by using a whispering gallery mode optical resonator formed of a dielectric material that allows for direct modulation of optical absorption by the electrical signal.

  17. Fabrication and optical characterization of Bragg resonance luminescence porous silicon

    NASA Astrophysics Data System (ADS)

    Park, Mi-Ae; Sohn, Honglae

    2016-01-01

    The synthesis and characterization of Bragg resonance luminescence porous silicon (BRL PS) exhibiting both optical reflectivity and strong narrow visible photoluminescence (PL) prepared from highly doped n-type silicon wafers through the electrochemical etching are reported. BRL PS showing the luminescence at 702 nm with an excitation wavelength of 400 nm was prepared by applying the current of 360 mA cm-2 for 1.6 s and 75 mA cm-2 for 3.6 s with 50 repeats in etching solution of 1:1 volume mixture of absolute ethanol and aqueous 48% HF. BRL PS exhibited sharp PL peak which reached full width at half maximum of 14 nm, originated from the result of Bragg resonance in PS multilayer. The sharp PL peak at 702 nm of BRL PS is the second-order transmitted luminescence peak by Bragg resonance phenomenon. The simultaneous measurement of reflectivity and luminescence in the BRL PS under an exposure to a vapor flux of acetone showed that a narrow transmitted luminescence based on Bragg resonance in BRL PS quenched as well as the red-shifted by 37 nm of reflection wavelength was observed. A dramatic quenching PL of BRL PS compare to that of the monolayer PS, is probably due to the Bragg resonance effect on luminescence.

  18. Resonance laser-plasma excitation of coherent terahertz phonons in the bulk of fluorine-bearing crystals under high-intensity femtosecond laser irradiation

    SciTech Connect

    Potemkin, F V; Mareev, E I; Khodakovskii, N G; Mikheev, P M

    2013-08-31

    The dynamics of coherent phonons in fluorine-containing crystals was investigated by pump-probe technique in the plasma production regime. Several phonon modes, whose frequencies are overtones of the 0.38-THz fundamental frequency, were simultaneously observed in a lithium fluoride crystal. Phonons with frequencies of 1 and 0.1 THz were discovered in a calcium fluoride crystal and coherent phonons with frequencies of 1 THz and 67 GHz were observed in a barium fluoride crystal. Furthermore, in the latter case the amplitudes of phonon mode oscillations were found to significantly increase 15 ps after laser irradiation. (interaction of laser radiation with matter)

  19. Cooling enhancement in optical refrigeration by non-resonant optical cavities

    NASA Astrophysics Data System (ADS)

    Farfan, B. G.; Gragossian, A.; Symonds, G.; Ghasemkhani, M. R.; Albrecht, A. R.; Sheik-Bahae, M.; Epstein, R. I.

    2016-05-01

    We present a study of cooling enhancement in optical refrigerators by the implementation of advanced non-resonant optical cavities. Cavity designs have been studied to maximize pump light-trapping to improve absorption and thereby increase the efficiency of optical refrigeration. The approaches of non-resonant optical cavities by Herriott-cell and totalinternal- reflection were studied. Ray-tracing simulations and experiments were performed to analyze and optimize the different light-trapping configurations. Light trapping was studied for laser sources with high quality beams and for beams with large divergences, roughly corresponding to the output from fiber lasers and from diode lasers, respectively. We present a trade-off analysis between performance, reliability, and manufacturability.

  20. Atomic-scale confinement of resonant optical fields.

    PubMed

    Kern, Johannes; Grossmann, Swen; Tarakina, Nadezda V; Häckel, Tim; Emmerling, Monika; Kamp, Martin; Huang, Jer-Shing; Biagioni, Paolo; Prangsma, Jord C; Hecht, Bert

    2012-11-14

    In the presence of matter, there is no fundamental limit preventing confinement of visible light even down to atomic scales. Achieving such confinement and the corresponding resonant intensity enhancement inevitably requires simultaneous control over atomic-scale details of material structures and over the optical modes that such structures support. By means of self-assembly we have obtained side-by-side aligned gold nanorod dimers with robust atomically defined gaps reaching below 0.5 nm. The existence of atomically confined light fields in these gaps is demonstrated by observing extreme Coulomb splitting of corresponding symmetric and antisymmetric dimer eigenmodes of more than 800 meV in white-light scattering experiments. Our results open new perspectives for atomically resolved spectroscopic imaging, deeply nonlinear optics, ultrasensing, cavity optomechanics, as well as for the realization of novel quantum-optical devices. PMID:22984927

  1. Spectral separation of optical spin based on antisymmetric Fano resonances

    PubMed Central

    Piao, Xianji; Yu, Sunkyu; Hong, Jiho; Park, Namkyoo

    2015-01-01

    We propose a route to the spectral separation of optical spin angular momentum based on spin-dependent Fano resonances with antisymmetric spectral profiles. By developing a spin-form coupled mode theory for chiral materials, the origin of antisymmetric Fano spectra is clarified in terms of the opposite temporal phase shift for each spin, which is the result of counter-rotating spin eigenvectors. An analytical expression of a spin-density Fano parameter is derived to enable quantitative analysis of the Fano-induced spin separation in the spectral domain. As an application, we demonstrate optical spin switching utilizing the extreme spectral sensitivity of the spin-density reversal. Our result paves a path toward the conservative spectral separation of spins without any need of the magneto-optical effect or circular dichroism, achieving excellent purity in spin density superior to conventional approaches based on circular dichroism. PMID:26561372

  2. Expansion of lower-frequency locally resonant band gaps using a double-sided stubbed composite phononic crystals plate with composite stubs

    NASA Astrophysics Data System (ADS)

    Li, Suobin; Chen, Tianning; Wang, Xiaopeng; Li, Yinggang; Chen, Weihua

    2016-06-01

    We studied the expansion of locally resonant complete band gaps in two-dimensional phononic crystals (PCs) using a double-sided stubbed composite PC plate with composite stubs. Results show that the introduction of the proposed structure gives rise to a significant expansion of the relative bandwidth by a factor of 1.5 and decreases the opening location of the first complete band gap by a factor of 3 compared to the classic double-sided stubbed PC plate with composite stubs. Furthermore, more band gaps appear in the lower-frequency range (0.006). These phenomena can be attributed to the strong coupling between the "analogous rigid mode" of the stub and the anti-symmetric Lamb modes of the plate. The "analogous rigid mode" of the stub is produced by strengthening the localized resonance effect of the composite plates through the double-sided stubs, and is further strengthened through the introduction of composite stubs. The "analogous rigid mode" of the stubs expands the out-of-plane band gap, which overlaps with in-plane band gap in the lower-frequency range. As a result, the complete band gap is expanded and more complete band gaps appear.

  3. Blue diode-pumped solid-state-laser based on ytterbium doped laser crystals operating on the resonance zero-phonon transition

    DOEpatents

    Krupke, William F.; Payne, Stephen A.; Marshall, Christopher D.

    2001-01-01

    The invention provides an efficient, compact means of generating blue laser light at a wavelength near .about.493+/-3 nm, based on the use of a laser diode-pumped Yb-doped laser crystal emitting on its zero phonon line (ZPL) resonance transition at a wavelength near .about.986+/-6 nm, whose fundamental infrared output radiation is harmonically doubled into the blue spectral region. The invention is applied to the excitation of biofluorescent dyes (in the .about.490-496 nm spectral region) utilized in flow cytometry, immunoassay, DNA sequencing, and other biofluorescence instruments. The preferred host crystals have strong ZPL fluorecence (laser) transitions lying in the spectral range from .about.980 to .about.992 nm (so that when frequency-doubled, they produce output radiation in the spectral range from 490 to 496 nm). Alternate preferred Yb doped tungstate crystals, such as Yb:KY(WO.sub.4).sub.2, may be configured to lase on the resonant ZPL transition near 981 nm (in lieu of the normal 1025 nm transition). The laser light is then doubled in the blue at 490.5 nm.

  4. Electro-optic ring resonators in integrated optics for miniature electric field sensors

    NASA Astrophysics Data System (ADS)

    Ruege, Alexander Charles

    This dissertation addresses two important aspects regarding the sensing of radio-frequency electromagnetic fields using integrated optical ring resonator devices. The first topic involves the theoretical design, fabrication and demonstration of a new field sensor based on electro-optically (EO) active integrated optical ring resonators. The second topic addresses the problem of enhancing the response from a single-mode ring resonator of a given ring waveguide loss through modifications in the device geometry. The miniature integrated optical EO ring resonator sensor consists of low-dielectric constant polymers, is metal-free and is supported by a thin, flexible substrate. The low-invasive platform is achieved through the development of a new fabrication process. The waveguide cores of the devices are constructed of polycarbonate doped with the EO chromophore Disperse Red 1 and are poled using the contact poling method. The measured loaded quality factors of the poled EO rings are between 15,600 and 18,900. The fields emanating from a microstrip resonator circuit at 3.9 GHz are measured. It is determined that the measured modulation from the four-ring linear array is largest when the optical wavelength is biased on the steep slopes of the resonance lineshapes as theoretically predicted. Using electric field values obtained from electromagnetic simulations of the microstrip circuit, the EO coefficient is 0.72 pm/V. The sensitivity for electric fields in free-space field is 142.2 V / (m Hz0.5). The sensitivity is obtained for an off-resonance optical power of -9 dBm at an optical wavelength near 1550 nm, a photoreceiver conversion gain of 900 V/W, and a system impedance of 50 ohm. Also, sensing from asymmetric lineshapes due to the bistable effect in the ring resonators is also demonstrated. This EO field sensing demonstration is the first reported using EO ring resonator sensors built on a metal-free flexible integrated optics platform. The second part of this

  5. Phase-sensitive optical detection of ballistic phonon heat pulses using frequency-modulation spectroscopy and persistent spectral holes

    NASA Astrophysics Data System (ADS)

    Ambrose, W. P.; Moerner, W. E.

    1991-01-01

    With the use of laser frequency-modulation (FM) spectroscopy and persistent spectral holes, time-resolved phase-sensitive probing of ballistic phonon heat pulses is accomplished in the interior of a NaF crystal. The ballistic phonon heat pulses are generated by the absorption of a Nd:YAG (neodymium-doped yttrium aluminum garnet) laser pulse in a Cr film on the sample surface. Local measurement of the propagating stress-strain field is illustrated by detecting the modulation of a spectral hole in the inhomogeneously broadened 607-nm color-center absorption in x-irradiated NaF at liquid-helium temperatures. By examining the dependence of the observed phonon time-of-flight data on the polarization of the probing light, the position within the sample, and the phase of FM detection, an identification of the acoustic polarizations of the propagating phonons may be made. The effects of phonon focusing and mode conversion upon reflection must be taken into account to complete the identification. Along with the ability to determine the sign of the acoustic disturbance, this experiment features a strain detection limit of 4×10-9 at a time resolution of 50 ns.

  6. Silicon Microdisk Resonators for Nonlinear Optics and Dynamics

    NASA Astrophysics Data System (ADS)

    Johnson, Thomas

    Silicon is incredibly well-studied as an electronic material. Since the out-migration of William Noyce, Gordon Moore, and the rest of the original Fairchild Semiconductor class from Shockley Semiconductor, silicon has only grown in prominence. Untold billions have been expended on research, development, and manufacture, and now silicon is perhaps the most well-controlled commercial material on Earth. For all that, the use of silicon as a mechanical material, though envisioned in the late 1950s, largely became viable only after the advent of large-scale silicon processing for microelectronics. As an optical material, silicon also has a long pedigree, with most of the positive focus on its excellent optical transparency and the enormous potential for improvement residing in its lack of effective emission. This thesis concerns an alternate route to the generation of light in silicon: the nonlinear route. Resonant elements play a critical role in making this viable. The ability to build up optical intensity in the confined volume of a microresonator reduces the input power required to achieve a given energy density. Silicon also has certain excellent nonlinear properties: a large Raman gain coefficient, for example, and an appreciable Kerr effect. Unfortunately, silicon also exhibits significant two-photon absorption (TPA) in the convenient telecommunications wavelength bands. As such, the build-up of optical energy in silion may also be accompanied by a build-up of TPA-induced free-carrier populations. These populations may serve to limit the efficiency of nonlinear processes or to generate additional nonlinear behavior in their interactions with optical fields. Thus two important stepping-stones on the way to the low-power, low-footprint use of silicon as an optical material are: the need to reduce optical losses in the optical elements, and to reduce or modify the populations of free carriers generated in the nonlinear optics regime. This thesis will present design

  7. Second harmonic generation by charge-transfer excitons interacting with phonons

    SciTech Connect

    Reineker, P.; Yudson, V. I.

    2001-06-15

    Effects of exciton-phonon interaction on the nonlinear optical response of charge-transfer excitons (CTE) are studied in the framework of an exactly solvable model. It is found that the second order excitonic optical polarizability {beta} is modified due to the CTE-phonon interaction. For a nonresonant frequency range, where {beta} is relatively small, the change is not significant. On the contrary, in the vicinity of resonances (when the light frequency {omega}{approximately}{omega}{sub 0} or {omega}{approximately}{omega}{sub 0}/2, {omega}{sub 0} is the CTE transition frequency), the CTE-phonon interaction may remarkably diminish the value of {beta}. This should be taken into account when considering CTE systems in nonlinear optics.

  8. 25th Anniversary Article: Ordered Polymer Structures for the Engineering of Photons and Phonons

    PubMed Central

    Lee, Jae-Hwang; Koh, Cheong Yang; Singer, Jonathan P; Jeon, Seog-Jin; Maldovan, Martin; Stein, Ori; Thomas, Edwin L

    2014-01-01

    The engineering of optical and acoustic material functionalities via construction of ordered local and global architectures on various length scales commensurate with and well below the characteristic length scales of photons and phonons in the material is an indispensable and powerful means to develop novel materials. In the current mature status of photonics, polymers hold a pivotal role in various application areas such as light-emission, sensing, energy, and displays, with exclusive advantages despite their relatively low dielectric constants. Moreover, in the nascent field of phononics, polymers are expected to be a superior material platform due to the ability for readily fabricated complex polymer structures possessing a wide range of mechanical behaviors, complete phononic bandgaps, and resonant architectures. In this review, polymer-centric photonic and phononic crystals and metamaterials are highlighted, and basic concepts, fabrication techniques, selected functional polymers, applications, and emerging ideas are introduced. PMID:24338738

  9. Observation of T2-like coherent optical phonons in epitaxial Ge2Sb2Te5/GaSb(001) films

    NASA Astrophysics Data System (ADS)

    Shalini, A.; Liu, Y.; Al-Jarah, U. A. S.; Srivastava, G. P.; Wright, C. D.; Katmis, F.; Braun, W.; Hicken, R. J.

    2013-10-01

    The phonon spectrum of Ge2Sb2Te5 is a signature of its crystallographic structure and underlies the phase transition process used in memory applications. Epitaxial materials allow coherent optical phonons to be studied in femtosecond anisotropic reflectance measurements. A dominant phonon mode with frequency of 3.4 THz has been observed in epitaxial Ge2Sb2Te5 grown on GaSb(001). The dependence of signal strength upon pump and probe polarization is described by a theory of transient stimulated Raman scattering that accounts for the symmetry of the crystallographic structure through use of the Raman tensor. The 3.4 THz mode has the character of the 3 dimensional T2 mode expected for the Oh point group, confirming that the underlying crystallographic structure is cubic. New modes are observed in both Ge2Sb2Te5 and GaSb after application of large pump fluences, and are interpreted as 1 and 2 dimensional modes associated with segregation of Sb.

  10. Observation of T2-like coherent optical phonons in epitaxial Ge2Sb2Te5/GaSb(001) films

    PubMed Central

    Shalini, A.; Liu, Y.; Al-Jarah, U.A.S.; Srivastava, G. P.; Wright, C. D.; Katmis, F.; Braun, W.; Hicken, R. J.

    2013-01-01

    The phonon spectrum of Ge2Sb2Te5 is a signature of its crystallographic structure and underlies the phase transition process used in memory applications. Epitaxial materials allow coherent optical phonons to be studied in femtosecond anisotropic reflectance measurements. A dominant phonon mode with frequency of 3.4 THz has been observed in epitaxial Ge2Sb2Te5 grown on GaSb(001). The dependence of signal strength upon pump and probe polarization is described by a theory of transient stimulated Raman scattering that accounts for the symmetry of the crystallographic structure through use of the Raman tensor. The 3.4 THz mode has the character of the 3 dimensional T2 mode expected for the Oh point group, confirming that the underlying crystallographic structure is cubic. New modes are observed in both Ge2Sb2Te5 and GaSb after application of large pump fluences, and are interpreted as 1 and 2 dimensional modes associated with segregation of Sb. PMID:24129388

  11. The influence of pyridine ligand onto the structure and phonon spectra of CdSe nanocrystals

    NASA Astrophysics Data System (ADS)

    Dzhagan, V. M.; Lokteva, I.; Himcinschi, C.; Kolny-Olesiak, J.; Valakh, M. Ya.; Schulze, S.; Zahn, D. R. T.

    2011-04-01

    The influence of ligand exchange for pyridine onto the structure and phonon spectra of oleic acid-stabilized CdSe nanocrystals (NCs) is studied by resonant Raman and optical absorption spectroscopy, nuclear magnetic resonance and transmission electron microscopy. The removal of oleic acid ligand by pyridine treatment results in change of intensity ratio of the longitudinal optical (LO) phonon peak to its overtones. The latter effect is attributed to a changed electron-phonon coupling in NCs upon introduction of the hole-capturing ligand (pyridine). The upward shift and broadening of the LO phonon peak are also observed and supposed to be the result of interplay between partial oxidation of the NC and strain induced by surface reconstruction. The relative contribution of these two effects is found to be dependent on the NC size. The activation of two additional Raman features, in the low-frequency range and above the LO band, for pyridine-treated NCs is supposed to be related with induced disorder or reconstruction on the NC surface. No noticeable effect of the surface treatment and concomitant NC aggregation onto the surface optical phonon mode was observed.

  12. Optical whispering-gallery mode resonators for applications in optical communication and frequency control

    NASA Astrophysics Data System (ADS)

    Grutter, Karen Esther

    High quality factor (Q) optical whispering gallery mode resonators are a key component in many on-chip optical systems, such as delay lines, modulators, and add-drop filters. They are also a convenient, compact structure for studying optomechanical interactions on-chip. In all these applications, optical Q is an important factor for high performance. For optomechanical reference oscillators in particular, high mechanical Q is also necessary. Previously, optical microresonators have been made in a wide variety of materials, but it has proven challenging to demonstrate high optical Q and high mechanical Q in a single, integrated device. This work demonstrates a new technique for achieving high optical Q on chip, a fully-integrated tunable filter with ultra-narrow minimum bandwidth, and the effect of material choice and device design on optical Q, mechanical Q and phase noise in microring optomechanical oscillators. To achieve a high optical Q, phosphosilicate glass (PSG) is studied as a resonator material. The low melting point of PSG enables wafer-scale reflow, which reduces sidewall roughness without significantly changing lithographically-defined dimensions. With this process, optical Qs up to 1.5 x 10. 7 are achieved, overten times higher than typical silicon optical resonators. These high-Q PSG resonators are then integrated with MEMS-actuated waveguides in a tunable-bandwidth filter. Due to the high Q of the PSG resonator, this device has a best-to-date minimum bandwidth of 0.8 GHz, with a tuning range of 0.8 to 8.5GHz. Finally, microring optomechanical oscillators (OMOs) in PSG, stoichiometric silicon nitride, and silicon are fabricated, and their performance is compared after characterization via a tapered optical fiber in vacuum. The silicon nitride device has the best performance, with a mechanical Q of more than 1 x 10. 4and record-breaking OMO phase noise of -102 dBc/Hz at a 1 kHz offset from a 72 MHz carrier.

  13. Miniature Trace Gas Detector Based on Microfabricated Optical Resonators

    NASA Technical Reports Server (NTRS)

    Aveline, David C.; Yu, Nan; Thompson, Robert J.; Strekalov, Dmitry V.

    2013-01-01

    While a variety of techniques exist to monitor trace gases, methods relying on absorption of laser light are the most commonly used in terrestrial applications. Cavity-enhanced absorption techniques typically use high-reflectivity mirrors to form a resonant cavity, inside of which a sample gas can be analyzed. The effective absorption length is augmented by the cavity's high quality factor, or Q, because the light reflects many times between the mirrors. The sensitivity of such mirror-based sensors scales with size, generally making them somewhat bulky in volume. Also, specialized coatings for the high-reflectivity mirrors have limited bandwidth (typically just a few nanometers), and the delicate mirror surfaces can easily be degraded by dust or chemical films. As a highly sensitive and compact alternative, JPL is developing a novel trace gas sensor based on a monolithic optical resonator structure that has been modified such that a gas sample can be directly injected into the cavity. This device concept combines ultra-high Q optical whispering gallery mode resonators (WGMR) with microfabrication technology used in the semiconductor industry. For direct access to the optical mode inside a resonator, material can be precisely milled from its perimeter, creating an open gap within the WGMR. Within this open notch, the full optical mode of the resonator can be accessed. While this modification may limit the obtainable Q, calculations show that the reduction is not significant enough to outweigh its utility for trace gas detection. The notch can be milled from the high- Q crystalline WGMR with a focused ion beam (FIB) instrument with resolution much finer than an optical wavelength, thereby minimizing scattering losses and preserving the optical quality. Initial experimental demonstrations have shown that these opened cavities still support high-Q whispering gallery modes. This technology could provide ultrasensitive detection of a variety of molecular species in an

  14. Micro-resonators coupled to atoms in an optical lattice

    NASA Astrophysics Data System (ADS)

    Geraci, Andrew; Kitching, John

    2010-03-01

    Recently there has been a convergence of ideas between the fields of solid-state and atomic physics -- examples range from using atoms for quantum simulation of condensed-matter Hamiltonians to physically coupling atoms with solid-state devices such as micro-resonators. In this talk, we discuss an experimental proposal involving an array of cooled microcantilevers coupled to a sample of ultracold atoms trapped near a microfabricated surface [1]. The cantilevers allow individual lattice site addressing for atomic state control and readout, and potentially may be useful in optical lattice quantum computation schemes. Assuming resonators can be cooled to their vibrational ground state, we describe the implementation of a two-qubit controlled-NOT gate with atomic internal states and the motional states of the resonators, along with a protocol for entangling two or more cantilevers on the atom chip using the trapped atoms as an intermediary. Although similar experiments could be carried out with magnetic microchip traps, the optical confinement scheme we consider may exhibit reduced near-field magnetic noise and decoherence. Prospects for using this system for tests of quantum mechanics at macroscopic scales or quantum information processing will be discussed. [4pt] [1] A. Geraci and J. Kitching, Phys. Rev. A 80, 032317 (2009)

  15. Optically Resonant Nanophotonic Devices for Label-Free Biomolecular Detection

    NASA Astrophysics Data System (ADS)

    Goddard, Julie; Mandal, Sudeep; Erickson, David

    Optical devices, such as surface plasmon resonance chips and waveguide-based Mach-Zehnder interferometers, have long been successfully used as label-free biomolecular sensors. Recently, however, there has been increased interest in developing new approaches to biomolecular detection that can improve on the limit of detection, specificity, and multiplexibility of these early devices and address emerging challenges in pathogen detection, disease diagnosis, and drug discovery. As we describe in this chapter, planar optically resonant nanophotonic devices (such as ring resonators, whispering gallery modes, and photonic crystal cavities) are one method that shows promise in significantly advancing the technology. Here we first provide a short review of these devices focusing on a handful of approaches illustrative of the state of the art. We then frame the major challenge to improving the technology as being the ability to provide simultaneously spatial localization of the electromagnetic energy and biomolecular binding events. We then introduce our “Nanoscale Optofluidic Sensor Arrays” which represents our approach to addressing this challenge. It is demonstrated how these devices serve to enable multiplexed detection while localizing the electromagnetic energy to a volume as small as a cubic wavelength. Challenges involved in the targeted immobilization of biomolecules over such a small area are discussed and our solutions presented. In general, we have tried to write this chapter with the novice in mind, providing details on the fabrication and immobilization methods that we have used and how one might adapt our approach to their designs.

  16. All-optical nonlinear plasmonic ring resonator switches

    NASA Astrophysics Data System (ADS)

    Nozhat, N.; Granpayeh, N.

    2014-11-01

    In this paper, all-optical nonlinear plasmonic ring resonator (PRR) switches containing 90o sharp and smooth bends have been proposed and numerically analyzed by the finite-difference time-domain method. Kerr nonlinear self-phase modulation (SPM) and cross-phase modulation (XPM) effects on the switching performance of the device have been studied. By applying a high-power lightwave, the signal can switch from one port to the other port due to the ON/OFF resonant states of the ring. We have shown that by utilizing the XPM effect, the output power ratio is improved by a factor of 2.5 and the required switching power is 31% of that of the case with only the SPM effect. Moreover, by utilizing sharp bend square-shaped ring resonators, the switching power is 10.4% lower than that of the smooth ones. The nonlinear PRR switches are suitable for application in photonic-integrated circuits as all-optical switches because of their nanoscale size and low required switching power.

  17. Optical phonon modes of III-V nanoparticles and indium phosphide/II-VI core-shell nanoparticles: A Raman and infrared study

    NASA Astrophysics Data System (ADS)

    Manciu, Felicia Speranta

    The prospects for realizing efficient nanoparticle light emitters in the visible/near IR for communications and bio-medical applications have benefited from progress in chemical fabrication of nanoparticles. III-V semiconductor nanopaticles such as GaP and InP are promising materials for the development of "blue" and "green" emitters, respectively, due to their large effective bandgaps. Enhanced emission efficiency has been achieved for core-shell nanoparticles, since inorganic shell materials increase electronic tunability and may decrease surface defects that often occur for nanoparticles capped with organic molecules. Also, the emission wavelength of InP nanoparticle cores can be tuned from green to red by changing the shell material in InP/II-VI core-shell nanoparticles. Investigations of phonon modes in nanocrystals are of both fundamental and applied interest. In the former case the optical phonon modes, such as surface/interface modes, are dependent on the nanoparticle dimensions, and also can provide information about dynamical properties of the nanoparticles and test the validity of various theoretical approaches. In the latter case the vibronic properties of nanoparticle emitters are controlled by confined phonons and modifications of the electron-phonon interaction by the confinement. Thus, the objective of the present thesis is the detailed study of the phonon modes of III-V nanoparticles (GaP and InP) and InP/II-VI core-shell nanoparticles by IR absorption and Raman scattering spectroscopies, and an elucidation of their complex vibrational properties. With the exception of three samples (two GaP and one InP), all samples were synthesized by a novel colloidal chemistry method, which does not requires added surfactant, but rather treatment of the corresponding precursors in octadecene noncoordinative solvent. Sample quality was characterized by ED, TEM and X-ray diffraction. Based on a comparison with a dielectric continuum model, the observed features

  18. On the fundamental mode of the optical resonator with toroidal mirrors

    SciTech Connect

    Serednyakov, S.S.; Vinokurov, N.A.

    1995-12-31

    The fundamental mode of the optical resonator with the toroidal mirrors is investigated. The losses in such resonator with the on-axis holes are low in compare with the case of spherical mirrors. The use of this type of optical resonator is briefly discussed.

  19. Resonance Raman Optical Activity of Single Walled Chiral Carbon Nanotubes.

    PubMed

    Nagy, Péter R; Koltai, János; Surján, Péter R; Kürti, Jenő; Szabados, Ágnes

    2016-07-21

    Resonance (vibrational) Raman Optical Activity (ROA) spectra of six chiral single-walled carbon nanotubes (SWCNTs) are studied by theoretical means. Calculations are performed imposing line group symmetry. Polarizability tensors, computed at the π-electron level, are differentiated with respect to DFT normal modes to generate spectral intensities. This computational protocol yields a ROA spectrum in good agreement with the only experiment on SWCNT, available at present. In addition to the conventional periodic electric dipole operator we introduce magnetic dipole and electric quadrupole operators, suitable for conventional k-space calculations. Consequences of the complex nature of the wave function on the scattering cross section are discussed in detail. The resonance phenomenon is accounted for by the short time approximation. Involvement of fundamental vibrations in the region of the intermediate frequency modes is found to be more notable in ROA than in Raman spectra. Calculations indicate exceptionally strong resonance enhancement of SWCNT ROA signals. Resonance ROA profile of the (6,5) tube shows an interesting sign change that may be exploited experimentally for SWCNT identification. PMID:27315548

  20. Statistics of chaotic resonances in an optical microcavity

    NASA Astrophysics Data System (ADS)

    Wang, Li; Lippolis, Domenico; Li, Ze-Yang; Jiang, Xue-Feng; Gong, Qihuang; Xiao, Yun-Feng

    2016-04-01

    Distributions of eigenmodes are widely concerned in both bounded and open systems. In the realm of chaos, counting resonances can characterize the underlying dynamics (regular vs chaotic), and is often instrumental to identify classical-to-quantum correspondence. Here, we study, both theoretically and experimentally, the statistics of chaotic resonances in an optical microcavity with a mixed phase space of both regular and chaotic dynamics. Information on the number of chaotic modes is extracted by counting regular modes, which couple to the former via dynamical tunneling. The experimental data are in agreement with a known semiclassical prediction for the dependence of the number of chaotic resonances on the number of open channels, while they deviate significantly from a purely random-matrix-theory-based treatment, in general. We ascribe this result to the ballistic decay of the rays, which occurs within Ehrenfest time, and importantly, within the time scale of transient chaos. The present approach may provide a general tool for the statistical analysis of chaotic resonances in open systems.

  1. Radiation-induced optic neuropathy: A magnetic resonance imaging study

    SciTech Connect

    Guy, J.; Mancuso, A.; Beck, R.; Moster, M.L.; Sedwick, L.A.; Quisling, R.G.; Rhoton, A.L. Jr.; Protzko, E.E.; Schiffman, J. )

    1991-03-01

    Optic neuropathy induced by radiation is an infrequent cause of delayed visual loss that may at times be difficult to differentiate from compression of the visual pathways by recurrent neoplasm. The authors describe six patients with this disorder who experienced loss of vision 6 to 36 months after neurological surgery and radiation therapy. Of the six patients in the series, two had a pituitary adenoma and one each had a metastatic melanoma, multiple myeloma, craniopharyngioma, and lymphoepithelioma. Visual acuity in the affected eyes ranged from 20/25 to no light perception. Magnetic resonance (MR) imaging showed sellar and parasellar recurrence of both pituitary adenomas, but the intrinsic lesions of the optic nerves and optic chiasm induced by radiation were enhanced after gadolinium-diethylenetriaminepenta-acetic acid (DTPA) administration and were clearly distinguishable from the suprasellar compression of tumor. Repeated MR imaging showed spontaneous resolution of gadolinium-DTPA enhancement of the optic nerve in a patient who was initially suspected of harboring recurrence of a metastatic malignant melanoma as the cause of visual loss. The authors found the presumptive diagnosis of radiation-induced optic neuropathy facilitated by MR imaging with gadolinium-DTPA. This neuro-imaging procedure may help avert exploratory surgery in some patients with recurrent neoplasm in whom the etiology of visual loss is uncertain.

  2. Relaxation times of the two-phonon processes with spin-flip and spin-conserving in quantum dots

    SciTech Connect

    Wang, Zi-Wu; Liu, Lei; Li, Shu-Shen

    2014-04-07

    We perform a theoretical investigation on the two-phonon processes of the spin-flip and spin-conserving relaxation in quantum dots in the frame of the Huang-Rhys' lattice relaxation model. We find that the relaxation time of the spin-flip is two orders of magnitude longer than that of the spin-conserving, which is in agreement with previous experimental measurements. Moreover, the opposite variational trends of the relaxation time as a function of the energy separation for two-phonon processes are obtained in different temperature regime. The relaxation times display the oscillatory behaviors at the demarcation point with increasing magnetic field, where the energy separation matches the optical phonon energy and results in the optical phonon resonance. These results are useful in understanding the intraband levels' relaxation in quantum dots and could be helpful in designing photoelectric and spin-memory devices.

  3. Structural polarization conversion in integrated optical vertically stacked ring resonators

    NASA Astrophysics Data System (ADS)

    Ciminelli, Caterina; Edoardo Campanella, Carlo; Nicola Armenise, Mario

    2013-06-01

    In this paper we report the structural polarization conversion effect occurring in an integrated optics device formed by two vertically stacked ring resonators excited through an underlying bus waveguide. We demonstrate that the vertical propagation of light, due to evanescent coupling, is enhanced by the resonant behavior of the device and the polarization state of a horizontally polarized input wave tends to be rotated within the device. In particular, a gradual polarization rotation can be observed when passing from one propagation plane to another, due to the geometry of the structure. This effect has been explained by taking into account all the physical mechanisms, which contribute to the polarization conversion. Although numerical results of general validity have been obtained, we also considered, as an example, silicon nitride technology due to its intrinsic features related to low cost and reduced technological problems.

  4. Optically Detected Ferromagnetic Resonance in Metallic Ferromagnets Via Off-Resonant Detection of Nitrogen Vacancy Centers in Diamond

    NASA Astrophysics Data System (ADS)

    Page, Michael R.; Bhallamudi, Vidya P.; Schulze, Joe; Purser, Carola M.; Manuilov, Sergei; Wolfe, Christopher; Brangham, Jack T.; Yang, Fengyuan; Hammel, P. Chris

    We report optical detection of ferromagnetic resonance in thin film metallic ferromagnets using a recently discovered approach employing nitrogen vacancy centers in nanodiamonds. While conventional optically detected magnetic resonance measures magnetic fields through their impact on the magnetic resonance frequency of the nitrogen vacancy center, we measure a change in the nitrogen vacancy center photoluminescence at the ferromagnet's resonance condition without need to work at the NV resonance frequency. This measurement technique allows sensitive, local detection of ferromagnetic resonance and can enable the study of magnetic dynamics at the nanoscale in a wide range of materials. While this measurement protocol was first reported in the study of ferromagnetic resonance in YIG, here we demonstrate the measurement in commonly used metallic ferromagnets to establish the generality of the technique and open the possibility of measuring nanoscale patterned devices and magnetic textures based on metallic ferromagnets of both commercial and scientific interest.

  5. Self-similarity and optical kinks in resonant nonlinear media

    SciTech Connect

    Ponomarenko, Sergey A.; Haghgoo, Soodeh

    2010-11-15

    We show that self-similar optical waves with a kink structure exist in a wide class of resonant nonlinear media, adequately treated in the two-level approximation. The self-similar structure of the present kinks is reflected in the time evolution of the field profile, atomic dipole moment, and one-atom inversion. We develop an analytical theory of such kinks. We show that the discovered kinks are accelerating nonlinear waves, asymptotically attaining their shape and the speed of light. We also numerically explore the formation and eventual disintegration of our kinks due to energy relaxation processes. Thus, the present kinks can be viewed as intermediate asymptotics of the system.

  6. Phononic Molecules Studied by Raman Scattering

    SciTech Connect

    Lanzillotti-Kimura, N. D.; Fainstein, A.; Jusserand, B.; Lemaitre, A.

    2010-01-04

    An acoustic nanocavity can confine phonons in such a way that they act like electrons in an atom. By combining two of these phononic-atoms, it is possible to form a phononic 'molecule', with acoustic modes that are similar to the electronic states in a hydrogen molecule. We report Raman scattering experiments performed in a monolithic structure formed by a phononic molecule embedded in an optical cavity. The acoustic mode splitting becomes evident through both the amplification and change of selection rules induced by the optical cavity confinement. The results are in perfect agreement with photoelastic model simulations.

  7. Optomechanical Enhancement of Doubly Resonant 2D Optical Nonlinearity.

    PubMed

    Yi, Fei; Ren, Mingliang; Reed, Jason C; Zhu, Hai; Hou, Jiechang; Naylor, Carl H; Johnson, A T Charlie; Agarwal, Ritesh; Cubukcu, Ertugrul

    2016-03-01

    Emerging two-dimensional semiconductor materials possess a giant second order nonlinear response due to excitonic effects while the monolayer thickness of such active materials limits their use in practical nonlinear devices. Here, we report 3300 times optomechanical enhancement of second harmonic generation from a MoS2 monolayer in a doubly resonant on-chip optical cavity. We achieve this by engineering the nonlinear light-matter interaction in a microelectro-mechanical system enabled optical frequency doubling device based on an electrostatically tunable Fabry-Perot microresonator. Our versatile optomechanical approach will pave the way for next generation efficient on-chip tunable light sources, sensors, and systems based on molecularly thin materials. PMID:26854706

  8. Resonant optical transducers for in-situ gas detection

    DOEpatents

    Bond, Tiziana C; Cole, Garrett; Goddard, Lynford

    2016-06-28

    Configurations for in-situ gas detection are provided, and include miniaturized photonic devices, low-optical-loss, guided-wave structures and state-selective adsorption coatings. High quality factor semiconductor resonators have been demonstrated in different configurations, such as micro-disks, micro-rings, micro-toroids, and photonic crystals with the properties of very narrow NIR transmission bands and sensitivity up to 10.sup.-9 (change in complex refractive index). The devices are therefore highly sensitive to changes in optical properties to the device parameters and can be tunable to the absorption of the chemical species of interest. Appropriate coatings applied to the device enhance state-specific molecular detection.

  9. Multiplex fiber-optic biosensor using multiple particle plasmon resonances

    NASA Astrophysics Data System (ADS)

    Lin, Hsing-Ying; Huang, Chen-Han; Liu, Yu-Chia; Huang, Kuo-Wei; Chau, Lai-Kwan

    2012-02-01

    Multiplex fiber-optic biosensor implemented by integrating multiple particle plasmon resonances (PPRs), molecular bioassays, and microfluidics is successfully demonstrated. The multiple PPRs are achieved by chemical immobilization of silver nanoparticles (AgNPs) and gold nanorods (AuNRs) separately on two unclad portions of an optical fiber. The difference in morphology and nature of material of AgNPs and AuNRs are exploited to yield multiple plasmonic absorptions at 405 and 780 nm in the absorption spectrum measured from optical fiber by white light source illumination. Through the coaxial excitation of light-emitting diodes (LEDs) with 405 and 800 nm wavelengths, the distinct PPRs are advantageous for real-time and simultaneous detection of multiple analyte-probe pairs as AgNPs and AuNRs are separately functionalized with specific bio-probes. Here, the multi-window fiber-optic particle plasmon resonance (FO-PPR) biosensor has been shown to be capable of simultaneously detecting anti-dinitrophenyl antibody (anti-DNP, MW = 220 kDa) via N-(2,4-dinitrophenyl)-6-aminohexanoic acid (DNP, MW = 297.27 Da) functionalized AgNPs and streptavidin (MW = 75 kDa) via N-(3-aminopropyl)biotinamide trifluoroacetate (biotin, MW = 414.44 Da) functionalized AuNRs. The multiplex sensing chip possesses several advantages, including rapid and parallel detection of multiple analytes on a single chip, minimized sample to sample variation, reduced amount of sensor chip, and reduced analyte volume, hence it is ideally suitable for high-throughput multiplex biochemical sensing applications.

  10. Characterization of the non-collinear acousto-optical cell based on calomel (Hg2Cl2) crystal and operating within the two-phonon light scattering

    NASA Astrophysics Data System (ADS)

    Shcherbakov, Alexandre S.; Arellanes, Adan O.

    2016-03-01

    Performances of any system for data processing based on acousto-optical technique are mainly determined by parameters of the acousto-optical cell (AOC) exploited within the schematic arrangement. Here, basic properties of the AOC, involved into a novel processor for precise optical spectrum analysis dedicated to modern astrophysical applications, are considered. Because potential applications of this processor will be focused on investigations in extra-galactic astronomy as well as studies of extra-solar planets, an advanced regime of the non-collinear two-phonon light scattering has been elaborated for spectrum analysis with significantly improved spectral resolution. Under similar uprated requirements, the AOC, based on that specific regime in the calomel (Hg2Cl2) crystal, had been chosen, and its parameters were analyzed theoretically and verified experimentally. Then, the adequate approach to estimating the frequency/spectral bandwidth and spectral resolution had been developed. The bandwidth was calculated and experimentally realized with the additionally involved tilt angle of light incidence, allowing variations for acoustic frequencies. The resolution was characterized taking into account its doubling peculiar to the nonlinear two-phonon mechanism of light scattering. Proof-of-principle experiments were performed with the calomel AOC of 52 mm optical aperture, providing ~94% efficiency in the transmitted light due to the slow-shear acoustic mode of finite amplitude (the acoustic power density ~150 mW/mm2) with the velocity of 0.347×105 cm/s at the radio-wave acoustic frequency ~71 MHz. As a result, we have obtained the spectral resolution <0.235 Å within the spectral bandwidth <290 Å that looks as the best one can mention at the moment in acousto-optics.

  11. Creating a zero-order resonator using an optical surface transformation.

    PubMed

    Sun, Fei; Ge, Xiaochen; He, Sailing

    2016-01-01

    A novel zero-order resonator has been designed by an optical surface transformation (OST) method. The resonator proposed here has many novel features. Firstly, the mode volume can be very small (e.g. in the subwavelength scale). Secondly, the resonator is open (no reflecting walls are utilized) and resonant effects can be found in a continuous spectrum (i.e. a continuum of eigenmodes). Thirdly, we only need one homogenous medium to realize the proposed resonator. The shape of the resonator can be a ring structure of arbitrary shape. In addition to the natural applications (e.g. optical storage) of an optical resonator, we also suggest some other applications of our novel optical open resonator (e.g. power combination, squeezing electromagnetic energy in the free space). PMID:26888359

  12. Creating a zero-order resonator using an optical surface transformation

    PubMed Central

    Sun, Fei; Ge, Xiaochen; He, Sailing

    2016-01-01

    A novel zero-order resonator has been designed by an optical surface transformation (OST) method. The resonator proposed here has many novel features. Firstly, the mode volume can be very small (e.g. in the subwavelength scale). Secondly, the resonator is open (no reflecting walls are utilized) and resonant effects can be found in a continuous spectrum (i.e. a continuum of eigenmodes). Thirdly, we only need one homogenous medium to realize the proposed resonator. The shape of the resonator can be a ring structure of arbitrary shape. In addition to the natural applications (e.g. optical storage) of an optical resonator, we also suggest some other applications of our novel optical open resonator (e.g. power combination, squeezing electromagnetic energy in the free space). PMID:26888359

  13. Tunable, continuous-wave single-resonant optical parametric oscillator with output coupling for resonant wave

    NASA Astrophysics Data System (ADS)

    Xiong-Hua, Zheng; Bao-Fu, Zhang; Zhong-Xing, Jiao; Biao, Wang

    2016-01-01

    We present a continuous-wave singly-resonant optical parametric oscillator with 1.5% output coupling of the resonant signal wave, based on an angle-polished MgO-doped periodically poled lithium niobate (MgO:PPLN), pumped by a commercial Nd:YVO4 laser at 1064 nm. The output-coupled optical parametric oscillator delivers a maximum total output power of 4.19 W with 42.8% extraction efficiency, across a tuning range of 1717 nm in the near- and mid-infrared region. This indicates improvements of 1.87 W in output power, 19.1% in extraction efficiency and 213 nm in tuning range extension in comparison with the optical parametric oscillator with no output coupling, while at the expense of increasing the oscillation threshold by a factor of ˜ 2. Moreover, it is confirmed that the finite output coupling also contributes to the reduction of the thermal effects in crystal. Project supported by the National Natural Science Foundation of China (Grant Nos. 61308056, 11204044, 11232015, and 11072271), the Research Fund for the Doctoral Program of Higher Education of China (Grant Nos. 20120171110005 and 20130171130003), the Fundamental Research Funds for the Central Universities of China (Grant No. 14lgpy07), and the Opening Project of Science and Technology on Reliability Physics and Application Technology of Electronic Component Laboratory, China (Grant No. ZHD201203).

  14. Integrated polymer micro-ring resonators for optical sensing applications

    NASA Astrophysics Data System (ADS)

    Girault, Pauline; Lorrain, Nathalie; Poffo, Luiz; Guendouz, Mohammed; Lemaitre, Jonathan; Carré, Christiane; Gadonna, Michel; Bosc, Dominique; Vignaud, Guillaume

    2015-03-01

    Micro-resonators (MR) have become a key element for integrated optical sensors due to their integration capability and their easy fabrication with low cost polymer materials. Nowadays, there is a growing need on MRs as highly sensitive and selective functions especially in the areas of food and health. The context of this work is to implement and study integrated micro-ring resonators devoted to sensing applications. They are fabricated by processing SU8 polymer as core layer and PMATRIFE polymer as lower cladding layer. The refractive index of the polymers and of the waveguide structure as a function of the wavelength is presented. Using these results, a theoretical study of the coupling between ring and straight waveguides has been undertaken in order to define the MR design. Sub-micronic gaps of 0.5 μm to 1 μm between the ring and the straight waveguides have been successfully achieved with UV (i-lines) photolithography. Different superstrates such as air, water, and aqueous solutions with glucose at different concentrations have been studied. First results show a good normalized transmission contrast of 0.98, a resonator quality factor around 1.5 × 104 corresponding to a coupling ratio of 14.7%, and ring propagation losses around 5 dB/cm. Preliminary sensing experiments have been performed for different concentrations of glucose; a sensitivity of 115 ± 8 nm/RIU at 1550 nm has been obtained with this couple of polymers.

  15. Origin invariance in vibrational resonance Raman optical activity.

    PubMed

    Vidal, Luciano N; Egidi, Franco; Barone, Vincenzo; Cappelli, Chiara

    2015-05-01

    A theoretical investigation on the origin dependence of the vibronic polarizabilities, isotropic and anisotropic rotational invariants, and scattering cross sections in Resonance Raman Optical Activity (RROA) spectroscopy is presented. Expressions showing the origin dependence of these polarizabilities were written in the resonance regime using the Franck-Condon (FC) and Herzberg-Teller (HT) approximations for the electronic transition moments. Differently from the far-from-resonance scattering regime, where the origin dependent terms cancel out when the rotational invariants are calculated, RROA spectrum can exhibit some origin dependence even for eigenfunctions of the electronic Hamiltonian. At the FC level, the RROA spectrum is completely origin invariant if the polarizabilities are calculated using a single excited state or for a set of degenerate states. Otherwise, some origin effects can be observed in the spectrum. At the HT level, RROA spectrum is origin dependent even when the polarizabilities are evaluated from a single excited state but the origin effect is expected to be small in this case. Numerical calculations performed for (S)-methyloxirane, (2R,3R)-dimethyloxirane, and (R)-4-F-2-azetidinone at both FC and HT levels using the velocity representation of the electric dipole and quadrupole transition moments confirm the predictions of the theory and show the extent of origin effects and the effectiveness of suggested ways to remove them. PMID:25956084

  16. Origin invariance in vibrational resonance Raman optical activity

    NASA Astrophysics Data System (ADS)

    Vidal, Luciano N.; Egidi, Franco; Barone, Vincenzo; Cappelli, Chiara

    2015-05-01

    A theoretical investigation on the origin dependence of the vibronic polarizabilities, isotropic and anisotropic rotational invariants, and scattering cross sections in Resonance Raman Optical Activity (RROA) spectroscopy is presented. Expressions showing the origin dependence of these polarizabilities were written in the resonance regime using the Franck-Condon (FC) and Herzberg-Teller (HT) approximations for the electronic transition moments. Differently from the far-from-resonance scattering regime, where the origin dependent terms cancel out when the rotational invariants are calculated, RROA spectrum can exhibit some origin dependence even for eigenfunctions of the electronic Hamiltonian. At the FC level, the RROA spectrum is completely origin invariant if the polarizabilities are calculated using a single excited state or for a set of degenerate states. Otherwise, some origin effects can be observed in the spectrum. At the HT level, RROA spectrum is origin dependent even when the polarizabilities are evaluated from a single excited state but the origin effect is expected to be small in this case. Numerical calculations performed for (S)-methyloxirane, (2R,3R)-dimethyloxirane, and (R)-4-F-2-azetidinone at both FC and HT levels using the velocity representation of the electric dipole and quadrupole transition moments confirm the predictions of the theory and show the extent of origin effects and the effectiveness of suggested ways to remove them.

  17. Sensitivity Improvement of Biosensors Using Si Ring Optical Resonators

    NASA Astrophysics Data System (ADS)

    Fukuyama, Masataka; Amemiya, Yoshiteru; Abe, Yosuke; Onishi, Yuto; Hirowatari, Anna; Terao, Kei; Ikeda, Takeshi; Kuroda, Akio; Yokoyama, Shin

    2011-04-01

    We have been demonstrating label-free detection of a variety of antigen-antibody reactions using Si ring optical resonators. Although the detection of biomarkers for the diagnosis of diseases generally requires high sensitivity of the order of 10-9 g/ml, the detection sensitivity of our device is currently of the order of 10-6 g/ml. In this paper, we show that the sensitivity of 10-9 g/ml will be possible by adopting the following four strategies: (1) use of slot-type waveguides with light wavelength of 1.3 µm, (2) improvement of quality factor Q of the ring resonator by smoothing the surface roughness, (3) specific adsorption of the bioreceptor protein to the resonator surface, and (4) maintaining temperature within ±0.005 °C. We have also proposed the on-chip temperature compensation method without the need for temperature control of the sample. By combining the proposed approaches, the sensitivity of the biosensor will be improved by a factor of >100, thus realizing practical application of our Si ring biosensor.

  18. Optical motion sensor for resonant-bar gravitational wave antennas.

    PubMed

    Richard, J P; Pang, Y; Hamilton, J J

    1992-04-01

    An experiment is described in which an optical method was used to measure fluctuations in the separation between two mirrors of a Fabry-Perot sensor cavity. Noise measurements were made to determine the sensitivity of this device to vibration amplitudes in the frequency range 1.1-2.1 kHz, which is of interestfor resonant-bar gravitational wave antennas. The rms spectral noise density for length fluctuations inthis range was 3.7 x 10(15-) m/Hz((1/2)) and can be related to electronic noise of the circuitry plus vibrationalnoise from the environment. The cavity finesse was relatively low at 117, and the power dissipated in the mirrors was estimated to be 1.9 muW. On a multimode gravitational wave detector, the sensor cavity would be formed by one reference mirror and by one mirror mounted on the last resonator. For a 1200-kg bar, 1.2-g last resonator system operating at 1600 Hz, the sensor described here would exhibit a noise temperature of 18 muK; the resolution in h in the case of negligible thermal noise from the mechanical system would be 3.7 x 10(-18)/Hz((1/2)). Improvements in the sensitivity in a quiet antenna-like environment should be possible with higher finesse mirrors. PMID:20720800

  19. Origin invariance in vibrational resonance Raman optical activity

    SciTech Connect

    Vidal, Luciano N. Cappelli, Chiara; Egidi, Franco; Barone, Vincenzo

    2015-05-07

    A theoretical investigation on the origin dependence of the vibronic polarizabilities, isotropic and anisotropic rotational invariants, and scattering cross sections in Resonance Raman Optical Activity (RROA) spectroscopy is presented. Expressions showing the origin dependence of these polarizabilities were written in the resonance regime using the Franck-Condon (FC) and Herzberg-Teller (HT) approximations for the electronic transition moments. Differently from the far-from-resonance scattering regime, where the origin dependent terms cancel out when the rotational invariants are calculated, RROA spectrum can exhibit some origin dependence even for eigenfunctions of the electronic Hamiltonian. At the FC level, the RROA spectrum is completely origin invariant if the polarizabilities are calculated using a single excited state or for a set of degenerate states. Otherwise, some origin effects can be observed in the spectrum. At the HT level, RROA spectrum is origin dependent even when the polarizabilities are evaluated from a single excited state but the origin effect is expected to be small in this case. Numerical calculations performed for (S)-methyloxirane, (2R,3R)-dimethyloxirane, and (R)-4-F-2-azetidinone at both FC and HT levels using the velocity representation of the electric dipole and quadrupole transition moments confirm the predictions of the theory and show the extent of origin effects and the effectiveness of suggested ways to remove them.

  20. Robust design of an optical router based on a tapered side-coupled integrated spaced sequence of optical resonators.

    PubMed

    Bettotti, P; Mancinelli, M; Guider, R; Masi, M; Vanacharla, M Rao; Pavesi, L

    2011-04-15

    A novel (to our knowledge) scheme of an optical router/switch element, composed of a tapered side-coupled integrated spaced sequence of optical resonators, is proposed. It is based on a modified design of the ring sequence in which the resonance conditions are set by the single ring resonance and by the coherent feedback of the sequence of rings. This double condition yields robustness against fabrication defects, dense routing capability, and high switching efficiency. PMID:21499394

  1. Rapid 3D µ-printing of polymer optical whispering-gallery mode resonators.

    PubMed

    Wu, Jushuai; Guo, Xin; Zhang, A Ping; Tam, Hwa-Yaw

    2015-11-16

    A novel microfabrication method for rapid printing of polymer optical whispering-gallery mode (WGM) resonators is presented. A 3D micro-printing technology based on high-speed optical spatial modulator (SLM) and high-power UV light source is developed to fabricate suspended-disk WGM resonator array using SU-8 photoresist. The optical spectral responses of the fabricated polymer WGM resonators were measured with a biconically tapered optical fiber. Experimental results reveal that the demonstrated method is very flexible and time-saving for rapid fabrication of complex polymer WGM resonators. PMID:26698452

  2. Phonon manipulation with phononic crystals.

    SciTech Connect

    Kim Bongsang; Hopkins, Patrick Edward; Leseman, Zayd C.; Goettler, Drew F.; Su, Mehmet F.; El-Kady, Ihab Fathy; Reinke, Charles M.; Olsson, Roy H., III

    2012-01-01

    In this work, we demonstrated engineered modification of propagation of thermal phonons, i.e. at THz frequencies, using phononic crystals. This work combined theoretical work at Sandia National Laboratories, the University of New Mexico, the University of Colorado Boulder, and Carnegie Mellon University; the MESA fabrication facilities at Sandia; and the microfabrication facilities at UNM to produce world-leading control of phonon propagation in silicon at frequencies up to 3 THz. These efforts culminated in a dramatic reduction in the thermal conductivity of silicon using phononic crystals by a factor of almost 30 as compared with the bulk value, and about 6 as compared with an unpatterned slab of the same thickness. This work represents a revolutionary advance in the engineering of thermoelectric materials for optimal, high-ZT performance. We have demonstrated the significant reduction of the thermal conductivity of silicon using phononic crystal structuring using MEMS-compatible fabrication techniques and in a planar platform that is amenable to integration with typical microelectronic systems. The measured reduction in thermal conductivity as compared to bulk silicon was about a factor of 20 in the cross-plane direction [26], and a factor of 6 in the in-plane direction. Since the electrical conductivity was only reduced by a corresponding factor of about 3 due to the removal of conductive material (i.e., porosity), and the Seebeck coefficient should remain constant as an intrinsic material property, this corresponds to an effective enhancement in ZT by a factor of 2. Given the number of papers in literature devoted to only a small, incremental change in ZT, the ability to boost the ZT of a material by a factor of 2 simply by reducing thermal conductivity is groundbreaking. The results in this work were obtained using silicon, a material that has benefitted from enormous interest in the microelectronics industry and that has a fairly large thermoelectric power

  3. Effect of Pure Dephasing and Phonon Scattering on the Coupling of Semiconductor Quantum Dots to Optical Cavities.

    PubMed

    Jarlov, C; Wodey, É; Lyasota, A; Calic, M; Gallo, P; Dwir, B; Rudra, A; Kapon, E

    2016-08-12

    Using site-controlled semiconductor quantum dots (QDs) free of multiexcitonic continuum states, integrated with photonic crystal membrane cavities, we clarify the effects of pure dephasing and phonon scattering on exciton-cavity coupling in the weak-coupling regime. In particular, the observed QD-cavity copolarization and cavity mode feeding versus QD-cavity detuning are explained quantitatively by a model of a two-level system embedded in a solid-state environment. PMID:27563983

  4. Effect of Pure Dephasing and Phonon Scattering on the Coupling of Semiconductor Quantum Dots to Optical Cavities

    NASA Astrophysics Data System (ADS)

    Jarlov, C.; Wodey, É.; Lyasota, A.; Calic, M.; Gallo, P.; Dwir, B.; Rudra, A.; Kapon, E.

    2016-08-01

    Using site-controlled semiconductor quantum dots (QDs) free of multiexcitonic continuum states, integrated with photonic crystal membrane cavities, we clarify the effects of pure dephasing and phonon scattering on exciton-cavity coupling in the weak-coupling regime. In particular, the observed QD-cavity copolarization and cavity mode feeding versus QD-cavity detuning are explained quantitatively by a model of a two-level system embedded in a solid-state environment.

  5. Temperature Dependence of Phonons in Pyrolitic Graphite

    DOE R&D Accomplishments Database

    Brockhouse, B. N.; Shirane, G.

    1977-01-01

    Dispersion curves for longitudinal and transverse phonons propagating along and near the c-axis in pyrolitic graphite at temperatures between 4°K and 1500°C have been measured by neutron spectroscopy. The observed frequencies decrease markedly with increasing temperature (except for the transverse optical ''rippling'' modes in the hexagonal planes). The neutron groups show interesting asymmetrical broadening ascribed to interference between one phonon and many phonon processes.

  6. Contactless ultrasound detection using an optical ring resonator

    NASA Astrophysics Data System (ADS)

    Kim, Kyu Hyun; Luo, Wei; Zhang, Cheng; Guo, L. Jay; Fan, Xudong

    2016-03-01

    We develop an air-couple ultrasound detector based on an optical fluidic ring resonator (OFRR) suspended on a Ushaped holder. The OFRR is a glass capillary with an outer diameter of approximately 130 μm and a wall thickness in the order of 1~10 μm. The circular cross section of the OFRR supports the high-Q whispering gallery mode (WGM) that circulates along the circumference. Incoming ultrasound pressure results in a small refractive index change in the glass wall and geometrical change in the OFRR shape, both of which in turn lead to a spectral shift in the WGM that can be sensitively detected owing to WGM with high optical Q-factors (>107). Due to the suspension nature of the OFRR, the ultrasound detection can be carried out in air, which is advantageous in comparison with other ultrasound detections that require acoustic coupling media such water, gel or solid. The sensitivity can be tuned and optimized by changing the diameter and wall thickness. Besides the optical detection, we also demonstrate optomechanical ultrasound mixing, in which optomechanical vibration is first excited within the OFRR that subsequently modulates the ultrasound wave. Our work will lead to the development of a new type of air-coupled ultrasound detector that can be used for photo-acoustic imaging, non-invasive ultrasound detection of external objects, and ultrasound detection/characterization of internal objects (such as particles and liquids) flowing inside the capillary.

  7. White-Light Whispering Gallery Mode Optical Resonator System and Method

    NASA Technical Reports Server (NTRS)

    Matsko, Andrey B. (Inventor); Savchenkov, Anatoliy A. (Inventor); Maleki, Lute (Inventor)

    2009-01-01

    An optical resonator system and method that includes a whispering-gallery mode (WGM) optical resonator that is capable of resonating across a broad, continuous swath of frequencies is provided. The optical resonator of the system is shaped to support at least one whispering gallery mode and includes a top surface, a bottom surface, a side wall, and a first curved transition region extending between the side wall and the top surface. The system further includes a coupler having a coupling surface which is arranged to face the transition region of the optical resonator and in the vicinity thereof such that an evanescent field emitted from the coupler is capable of being coupled into the optical resonator through the first curved transition region

  8. Studying an advanced regime of the non-collinear two-phonon light scattering for applications to the optical spectrum analysis

    NASA Astrophysics Data System (ADS)

    Shcherbakov, Alexandre S.; Arellanes, Adan O.

    2016-03-01

    Principally new features of the non-collinear two-phonon light scattering governed by elastic waves of finite amplitude in birefringent bulk crystals are detected and observed. The main goals of our investigations are to reveal novel important details inherent in the nonlinearity of this effect and to study properties of similar parametric nonlinearity both theoretically and experimentally in wide-aperture crystals with moderate linear acoustic attenuation. An additional degree of freedom represented by the dispersive birefringence factor, which can be distinguished within this nonlinear phenomenon, is characterized. This physical degree of freedom gives us a one-of-a-kind opportunity to apply the strongly non-linear two-phonon light scattering in practice for the first time. The local unit-level maxima in the distribution of light scattered into the second order appear periodically as the acoustic power density grows. It makes possible to identify a few transfer function profiles peculiar to these maxima in the isolated planes of angular-frequency mismatches. These maxima give us an opportunity to choose the desirable profile for the transfer function at the fixed angle of incidence for the incoming light beam with a wide spectrum .The needed theoretical analysis is developed and proof-of-principle experiments, performed with a specially designed wide-aperture acousto-optical cell made of the calomel (α-Hg2Cl2) crystal, are presented. The obtained spectral resolution ~0.235 Å at 405 nm (i.e. the resolving power ~17,200) can be compared with the most advanced acousto-optical spectrometers for space/airborne operations. Evidently, our results with the calomel-based acousto-optical cell look like the best we can mention at the moment.

  9. Tapered Optical Fibers Designed for Surface Plasmon Resonance Phase Matching

    PubMed Central

    Yu, Yinni; Blake, Phillip; Roper, D. Keith

    2009-01-01

    Combining a modified two-step chemical etch method with equations to predict etch parameters and photon-plasmon phase-matching resulted in single-mode tapered optical fibers (TOFs) to optimize electromagnetic field enhancement. The phase-matching equation was used to identify the angle of incidence near the TOF cutoff radius at which surface plasmon resonance (SPR) is maximized. The axisymmetric Young–Laplace equation was used to predict the angle of incidence from the fabrication of a TOF via chemical etching. An optimal cone angle of 20.0°, angles of incidence averaging (81.6 ± 1.9)°, and tip diameters of (80.0 ± 14.1) nm were achieved through a two-step etching process. These TOF characteristics maximize SPR excitation and field enhancement. The refractive index for optimized SPR excitation in the fabricated TOFs at a wavelength of 650 nm was found to be 1.343. PMID:19061312

  10. Brain metastasis detection by resonant Raman optical biopsy method

    NASA Astrophysics Data System (ADS)

    Zhou, Yan; Liu, Cheng-hui; Cheng, Gangge; Zhou, Lixin; Zhang, Chunyuan; Pu, Yang; Li, Zhongwu; Liu, Yulong; Li, Qingbo; Wang, Wei; Alfano, Robert R.

    2014-03-01

    Resonant Raman (RR) spectroscopy provides an effective way to enhance Raman signal from particular bonds associated with key molecules due to changes on a molecular level. In this study, RR is used for detection of human brain metastases of five kinds of primary organs of lung, breast, kidney, rectal and orbital in ex-vivo. The RR spectra of brain metastases cancerous tissues were measured and compared with those of normal brain tissues and the corresponding primary cancer tissues. The differences of five types of brain metastases tissues in key bio-components of carotene, tryptophan, lactate, alanine and methyl/methylene group were investigated. The SVM-KNN classifier was used to categorize a set of RR spectra data of brain metastasis of lung cancerous tissues from normal brain tissue, yielding diagnostic sensitivity and specificity at 100% and 75%, respectively. The RR spectroscopy may provide new moleculebased optical probe tools for diagnosis and classification of brain metastatic of cancers.

  11. Optomechanically induced stochastic resonance and chaos transfer between optical fields

    NASA Astrophysics Data System (ADS)

    Monifi, Faraz; Zhang, Jing; Özdemir, Şahin Kaya; Peng, Bo; Liu, Yu-Xi; Bo, Fang; Nori, Franco; Yang, Lan

    2016-06-01

    Chaotic dynamics has been reported in many physical systems and has affected almost every field of science. Chaos involves hypersensitivity to the initial conditions of a system and introduces unpredictability into its output. Thus, it is often unwanted. Interestingly, the very same features make chaos a powerful tool to suppress decoherence, achieve secure communication and replace background noise in stochastic resonance—a counterintuitive concept that a system's ability to transfer information can be coherently amplified by adding noise. Here, we report the first demonstration of chaos-induced stochastic resonance in an optomechanical system, as well as the optomechanically mediated chaos transfer between two optical fields such that they follow the same route to chaos. These results will contribute to the understanding of nonlinear phenomena and chaos in optomechanical systems, and may find applications in the chaotic transfer of information and for improving the detection of otherwise undetectable signals in optomechanical systems.

  12. Optical Manipulation and Spectroscopy Of Silicon Nanoparticles Exhibiting Dielectric Resonances.

    PubMed

    Andres-Arroyo, Ana; Gupta, Bakul; Wang, Fan; Gooding, J Justin; Reece, Peter J

    2016-03-01

    We demonstrate that silicon (Si) nanoparticles with scattering properties exhibiting strong dielectric resonances can be successfully manipulated using optical tweezers. The large dielectric constant of Si has a distinct advantage over conventional colloidal nanoparticles in that it leads to enhanced trapping forces without the heating associated with metallic nanoparticles. Further, the spectral features of the trapped nanoparticles provide a unique marker for probing size, shape, orientation and local dielectric environment. We exploit these properties to investigate the trapping dynamics of Si nanoparticles with different dimensions ranging from 50 to 200 nm and aspect ratios between 0.4 and 2. The unique combination of spectral and trapping properties make Si nanoparticles an ideal system for delivering directed nanoscale sensing in a range of potential applications. PMID:26848883

  13. Optical and electrical properties and phonon drag effect in low temperature TEP measurements of AgSbSe2 thin films

    NASA Astrophysics Data System (ADS)

    Namitha Asokan, T.; Urmila, K. S.; Jacob, Rajani; Reena Philip, Rachel; Okram, G. S.; Ganesan, V.; Pradeep, B.

    2014-05-01

    Polycrystalline thin films of silver antimony selenide have been deposited using a reactive evaporation technique onto an ultrasonically cleaned glass substrate at a vacuum of 10-5 torr. The preparative parameters, like substrate temperature and incident fluxes, have been properly controlled in order to get stoichiometric, good quality and reproducible thin film samples. The samples are characterized by XRD, SEM, AFM and a UV—vis—NIR spectrophotometer. The prepared sample is found to be polycrystalline in nature. From the XRD pattern, the average particle size and lattice constant are calculated. The dislocation density, strain and number of crystallites per unit area are evaluated using the average particle size. The dependence of the electrical conductivity on the temperature has also been studied and the prepared AgSbSe2 samples are semiconducting in nature. The AgSbSe2 thin films exhibited an indirect allowed optical transition with a band gap of 0.64 eV. The compound exhibits promising thermoelectric properties, a large Seebeck coefficient of 30 mV/K at 48 K due to strong phonon electron interaction. It shows a strong temperature dependence on thermoelectric properties, including the inversion of a dominant carrier type from p to n over a low temperature range 9-300 K, which is explained on the basis of a phonon drag effect.

  14. Quasi-static high-resolution magnetic-field detection based on dielectric optical resonators

    NASA Astrophysics Data System (ADS)

    Ioppolo, Tindaro; Rubino, Edoardo

    2013-06-01

    In this paper we present a high resolution magnetic field sensor that is based on the perturbation of the optical modes (whispering gallery mode, WGM) of a spherical dielectric resonator. The optical resonator is side coupled to a tapered single mode optical fiber. One side of the optical fiber is coupled to a distribute feedback diode laser, while the other end is connected to a photodiode. The optical modes of the dielectric cavity are perturbed using a metglas sheet that is in contact with the resonator. When the metglas sheet is exposed to an external magnetic field it elongates perturbing the optical modes of the dielectric cavity. This in turn leads to a shift in the optical resonances. By measuring the induced WGM shift the magnetic field can be measured. Preliminary results show sensor resolution of a few nanoteslas.

  15. Performance of resonator fiber optic gyroscope using external-cavity laser stabilization and optical filtering

    NASA Astrophysics Data System (ADS)

    Qiu, Tiequn; Wu, Jianfeng; Strandjord, Lee K.; Sanders, Glen A.

    2014-05-01

    A bench-top resonator fiber optic gyroscope (RFOG) was assembled and tested, showing encouraging progress toward navigation grade performance. The gyro employed a fiber length of 19 meters of polarizing fiber for the sensing coil which was wound on an 11.5 cm diameter PZT cylinder. A bias stability of approximately 0.1 deg/hr was observed over a 2 hour timeframe, which is the best bias stability reported to date in an RFOG to our knowledge. Special care was taken to minimize laser phase noise, including stabilization to an optical cavity which was also used for optical filtering, giving angle random walk (ARW) values in the range of 0.008 deg/rt-hr. The ARW performance and bias stability are within 2x and 10x, respectively, of many civil inertial navigation grade requirements.

  16. Watching surface waves in phononic crystals.

    PubMed

    Wright, Oliver B; Matsuda, Osamu

    2015-08-28

    In this paper, we review results obtained by ultrafast imaging of gigahertz surface acoustic waves in surface phononic crystals with one- and two-dimensional periodicities. By use of quasi-point-source optical excitation, we show how, from a series of images that form a movie of the travelling waves, the dispersion relation of the acoustic modes, their corresponding mode patterns and the position and widths of phonon stop bands can be obtained by temporal and spatio-temporal Fourier analysis. We further demonstrate how one can follow the temporal evolution of phononic eigenstates in k-space using data from phononic-crystal waveguides as an example. PMID:26217053

  17. Plasmonic Resonant Absorption in Mid-Infrared in Graphene Nanoresonators

    NASA Astrophysics Data System (ADS)

    Abeysinghe, Don C.; Myers, Joshua; Esfahani, Nima N.; Walker, Dennis E., Jr.; Hendrickson, Joshua R.; Cleary, Justin; Mou, Shin; Air Force Research Laboratory, Materials; Manufacturing Directorate, Wright-Patterson AFB, OH, USA Team; Air Force Research Laboratory, Sensors Directorate, Wright-Patterson AFB, OH, USA Team

    2014-03-01

    We experimentally demonstrated polarization-sensitive, tunable plasmonic resonant absorption in the mid-infrared range of 5-14 um by utilizing an array of graphene nanoribbon resonators. By tuning resonator width and charge density, we probed graphene plasmons with λp <= λ /100 and plasmon resonance energy as high as 0.26 meV (2100 cm-1) for 40 nm wide nanoresonators. Resonant absorption spectra enabled us to map the wavevector-frequency dispersion for graphene plasmons at mid-IR energies and revealed a modified plasmon dispersion as well as plasmon damping due to intrinsic optical phonons of graphene and graphene plasmon interaction with the surface polar phonons in SiO2 substrates. Additionally, we studied spectra further by introducing intrinsic defect phonons and doping by direct electron beam irradiation of graphene nanoresonators

  18. High-sensitivity optical monitoring of a micromechanical resonator with a quantum-limited optomechanical sensor.

    PubMed

    Arcizet, O; Cohadon, P-F; Briant, T; Pinard, M; Heidmann, A; Mackowski, J-M; Michel, C; Pinard, L; Français, O; Rousseau, L

    2006-09-29

    We experimentally demonstrate the high-sensitivity optical monitoring of a micromechanical resonator and its cooling by active control. Coating a low-loss mirror upon the resonator, we have built an optomechanical sensor based on a very high-finesse cavity (30 000). We have measured the thermal noise of the resonator with a quantum-limited sensitivity at the 10(-19) m/sqrt[Hz] level, and cooled the resonator down to 5 K by a cold-damping technique. Applications of our setup range from quantum optics experiments to the experimental demonstration of the quantum ground state of a macroscopic mechanical resonator. PMID:17026032

  19. Novel localized surface plasmon resonance based optical fiber sensor

    NASA Astrophysics Data System (ADS)

    Muri, Harald Ian D. I.; Hjelme, Dag R.

    2016-03-01

    Over the last decade various optical fiber sensing schemes have been proposed based on local surface plasmon resonance (LSPR). LSPR are interacting with the evanescent field from light propagating in the fiber core or by interacting with the light at the fiber end face. Sensor designs utilizing the fiber end face is strongly preferred from a manufacturing point of view. However, the different techniques available to immobilize metallic nanostructures on the fiber end face for LSPR sensing is limited to essentially a monolayer, either by photolithographic structuring of metal film, thermal nucleation of metal film, or by random immobilization of nanoparticles (NP). In this paper, we report on a novel LSPR based optical fiber sensor architecture. The sensor is prepared by immobilizing gold NP's in a hydrogel droplet polymerized on the fiber end face. This design has several advantages over earlier designs. It dramatically increase the number of NP's available for sensing, it offers precise control over the NP density, and the NPs are position in a true 3D aqueous environment. The sensor design is also compatible with low cost manufacturing. The sensor design can measure volumetric changes in a stimuli-responsive hydrogel or measure binding to receptors on the NP surface. It can also be used as a two-parameter sensor by utilizing both effects. We present results from proof-of-concept experiments demonstrating a pH sensor based on LSPR sensing in a poly(acrylamide-co-acrylic acid) hydrogel embedding gold nanoparticles.

  20. [Optical surface plasmon resonance biosensors in molecular fishing].

    PubMed

    Ivanov, A S; Medvedev, A E

    2015-01-01

    An optical biosensor employing surface plasmon resonance is a highly efficient instrument applicable for direct real time registration of molecular interactions without additional use of any labels or coupled processes. As an independent approach it is especially effective in analysis of various ligand receptor interactions. SPR-biosensors are used for validation of studies on intermolecular interactions in complex biological systems (affinity profiling of various groups of proteins, etc.). Recently, potential application of the SPR-biosensor for molecular fishing (direct affinity binding of target molecules from complex biological mixtures on the optical biosensor surface followed by their elution for identification by LC-MS/MS) has been demonstrated. Using SPR-biosensors in such studies it is possible to solve the following tasks: (a) SPR-based selection of immobilization conditions required for the most effective affinity separation of a particular biological sample; (b) SPR-based molecular fishing for subsequent protein identification by mass spectrometry; (c) SPR-based validation of the interaction of identified proteins with immobilized ligand. This review considers practical application of the SPR technology in the context of recent studies performed in the Institute of Biomedical Chemistry on molecular fishing of real biological objects. PMID:25978389

  1. Phononic crystal devices

    DOEpatents

    El-Kady, Ihab F.; Olsson, Roy H.

    2012-01-10

    Phononic crystals that have the ability to modify and control the thermal black body phonon distribution and the phonon component of heat transport in a solid. In particular, the thermal conductivity and heat capacity can be modified by altering the phonon density of states in a phononic crystal. The present invention is directed to phononic crystal devices and materials such as radio frequency (RF) tags powered from ambient heat, dielectrics with extremely low thermal conductivity, thermoelectric materials with a higher ratio of electrical-to-thermal conductivity, materials with phononically engineered heat capacity, phononic crystal waveguides that enable accelerated cooling, and a variety of low temperature application devices.

  2. Optical pulling force and conveyor belt effect in resonator-waveguide system.

    PubMed

    Intaraprasonk, Varat; Fan, Shanhui

    2013-09-01

    We present the theoretical condition and actual numerical design that achieves an optical pulling force in resonator-waveguide systems, where the direction of the force on the resonator is in the opposite direction to the input light in the waveguide. We also show that this pulling force can occur in conjunction with the lateral optical equilibrium effect, such that the resonator is maintained at the fixed distance from the waveguide while experiencing the pulling force. PMID:23988930

  3. Lasing from active optomechanical resonators.

    PubMed

    Czerniuk, T; Brüggemann, C; Tepper, J; Brodbeck, S; Schneider, C; Kamp, M; Höfling, S; Glavin, B A; Yakovlev, D R; Akimov, A V; Bayer, M

    2014-01-01

    Planar microcavities with distributed Bragg reflectors (DBRs) host, besides confined optical modes, also mechanical resonances due to stop bands in the phonon dispersion relation of the DBRs. These resonances have frequencies in the 10- to 100-GHz range, depending on the resonator's optical wavelength, with quality factors exceeding 1,000. The interaction of photons and phonons in such optomechanical systems can be drastically enhanced, opening a new route towards the manipulation of light. Here we implemented active semiconducting layers into the microcavity to obtain a vertical-cavity surface-emitting laser (VCSEL). Thereby, three resonant excitations--photons, phonons and electrons--can interact strongly with each other providing modulation of the VCSEL laser emission: a picosecond strain pulse injected into the VCSEL excites long-living mechanical resonances therein. As a result, modulation of the lasing intensity at frequencies up to 40 GHz is observed. From these findings, prospective applications of active optomechanical resonators integrated into nanophotonic circuits may emerge. PMID:25008784

  4. Backscattering analysis in optical micro-resonators with mode splitting based on COMSOL

    NASA Astrophysics Data System (ADS)

    Yang, Zhaohua; Huo, Jiayan; Yang, Xu

    2015-10-01

    Rayleigh backscattering noise, which is one of the reasons that limit the sensitivity, has been deemed as noise in traditional resonant optic gyroscopes. However Rayleigh backscattering noise is one of the incentives of mode splitting phenomenon in high-Q resonators. Regarding the change of the resonance frequency of the resonator caused by the scattering signal as a measurement, we can use mode splitting to measure temperature, size of nanoparticle, etc. Light is confined by total internal reflection in whispering gallery mode (WGM) optical resonators, which is characterized by high-Q factors and small mode volumes. With regards to this, we propose a sensing mechanism based on mode splitting in high-Q WGM optical resonators. It is possible for us to measure the angular velocity of carrier according to the changes in the resonant frequencies of the two splitting modes. We propose the Miniature resonant optic gyroscope based on mode splitting (MROG-MS) with WGM resonators in the paper. Considering the Sagnac effect, mode splitting in high quality optical micro-resonators, and the rotation-induced impact on backscattering process, we modify the equations of motion that describe mode splitting, derive the explicit expression of angular rate versus the splitting amount, and verify the sensing mechanism by the simulation based on COMSOL. Furthermore, after monitoring the transmission spectra at different number of scattering particles, the simulation shows that mode splitting phenomenon resulted by single particle is more suitable for angular velocity measurement.

  5. Optically-Switched Resonant Tunneling Diodes for Space-Based Optical Communication Applications

    NASA Technical Reports Server (NTRS)

    Moise, T. S.; Kao, Y. -C.; Jovanovic, D.; Sotirelis, P.

    1995-01-01

    We are developing a new type of digital photo-receiver that has the potential to perform high speed optical-to-electronic conversion with a factor of 10 reduction in component count and power dissipation. In this paper, we describe the room-temperature photo-induced switching of this InP-based device which consists of an InGaAs/AlAs resonant tunneling diode integrated with an InGaAs absorber layer. When illuminated at an irradiance of greater than 5 Wcm(exp -2) using 1.3 micromillimeter radiation, the resonant tunneling diode switches from a high-conductance to a low-conductance electrical state and exhibits a voltage swing of up to 800 mV.

  6. Integrated optics ring-resonator chemical sensor with polymer transduction layer

    NASA Technical Reports Server (NTRS)

    Ksendzov, A.; Homer, M. L.; Manfreda, A. M.

    2004-01-01

    An integrated optics chemical sensor based on a ring resonator with an ethyl cellulose polymer coating has been demonstrated. The measured sensitivity to isopropanol in air is 50 ppm-the level immediately useful for health-related air quality monitoring. The resonator was fabricated using SiO2 and SixNy materials. The signal readout is based on tracking the wavelength of a resonance peak. The resonator layout optimisation for sensing applications is discussed.

  7. Analysis of resonant optical gyroscopes with two input/output waveguides.

    PubMed

    Hah, Dooyoung; Zhang, Dan

    2010-08-16

    Rotation sensitivity of optical gyroscopes with ring resonators and two input/output waveguides in a coplanar add-drop filter configuration is studied. First, the gyroscope with a single resonator is analyzed, which is shown to have slightly higher sensitivity than the one with one waveguide. Next, the sensor with two identical resonators coupled through waveguides is investigated, which turns out to have half the sensitivity of the one with a single resonator when compared for the same footprints. The last point is valid when the resonators have the same coupling coefficients to the waveguides in the sensor with two resonators. PMID:20721209

  8. Enhancement of the transverse magneto-optical Kerr effect via resonant tunneling in trilayers containing magneto-optical metals

    NASA Astrophysics Data System (ADS)

    Girón-Sedas, J. A.; Mejía-Salazar, J. R.; Moncada-Villa, E.; Porras-Montenegro, N.

    2016-07-01

    We propose a way to enhance the transverse magneto-optical Kerr effect, by the excitation of resonant tunneling modes, in subwavelength trilayer structures featuring a dielectric slab sandwiched between two magneto-optical metallic layers. Depending on the magneto-optical layer widths, the proposed system may exhibit an extraordinary transverse magneto-optical Kerr effect, which makes it very attractive for the design and engineering of thin-film magneto-optical-based devices for future photonic circuits or fiber optical-communication systems.

  9. Studies of Phonon Anharmonicity in Solids

    NASA Astrophysics Data System (ADS)

    Lan, Tian

    Today our understanding of the vibrational thermodynamics of materials at low temperatures is emerging nicely, based on the harmonic model in which phonons are independent. At high temperatures, however, this understanding must accommodate how phonons interact with other phonons or with other excitations. We shall see that the phonon-phonon interactions give rise to interesting coupling problems, and essentially modify the equilibrium and non-equilibrium properties of materials, e.g., thermodynamic stability, heat capacity, optical properties and thermal transport of materials. Despite its great importance, to date the anharmonic lattice dynamics is poorly understood and most studies on lattice dynamics still rely on the harmonic or quasiharmonic models. There have been very few studies on the pure phonon anharmonicity and phonon-phonon interactions. The work presented in this thesis is devoted to the development of experimental and computational methods on this subject. Modern inelastic scattering techniques with neutrons or photons are ideal for sorting out the anharmonic contribution. Analysis of the experimental data can generate vibrational spectra of the materials, i.e., their phonon densities of states or phonon dispersion relations. We obtained high quality data from laser Raman spectrometer, Fourier transform infrared spectrometer and inelastic neutron spectrometer. With accurate phonon spectra data, we obtained the energy shifts and lifetime broadenings of the interacting phonons, and the vibrational entropies of different materials. The understanding of them then relies on the development of the fundamental theories and the computational methods. We developed an efficient post-processor for analyzing the anharmonic vibrations from the molecular dynamics (MD) calculations. Currently, most first principles methods are not capable of dealing with strong anharmonicity, because the interactions of phonons are ignored at finite temperatures. Our method adopts

  10. Fano resonance-induced negative optical scattering force on plasmonic nanoparticles.

    PubMed

    Chen, Huajin; Liu, Shiyang; Zi, Jian; Lin, Zhifang

    2015-02-24

    We demonstrate theoretically that Fano resonance can induce a negative optical scattering force acting on plasmonic nanoparticles in the visible light spectrum when an appropriate manipulating laser beam is adopted. Under the illumination of a zeroth-order Bessel beam, the plasmonic nanoparticle at its Fano resonance exhibits a much stronger forward scattering than backward scattering and consequently leads to a net longitudinal backward optical scattering force, termed Fano resonance-induced negative optical scattering force. The extinction spectra obtained based on the Mie theory show that the Fano resonance arises from the interference of simultaneously excited multipoles, which can be either a broad electric dipole mode and a narrow electric quadrupole mode, or a quadrupole and an octupole mode mediated by the broad electric dipole. Such Fano resonance-induced negative optical scattering force is demonstrated to occur for core-shell, homogeneous, and hollow metallic particles and can therefore be expected to be universal for many other nanostructures exhibiting Fano resonance, adding considerably to the flexibility of optical micromanipulation on the plasmonic nanoparticles. More interestingly, the flexible tunability of the Fano resonance by particle morphology opens up the possibility of tailoring the optical scattering force accordingly, offering an additional degree of freedom to optical selection and sorting of plasmonic nanoparticles. PMID:25635617

  11. Frequency stabilization of the zero-phonon line of a quantum dot via phonon-assisted active feedback

    SciTech Connect

    Hansom, Jack; Schulte, Carsten H. H.; Matthiesen, Clemens; Stanley, Megan J.; Atatüre, Mete

    2014-10-27

    We report on the feedback stabilization of the zero-phonon emission frequency of a single InAs quantum dot. The spectral separation of the phonon-assisted component of the resonance fluorescence provides a probe of the detuning between the zero-phonon transition and the resonant driving laser. Using this probe in combination with active feedback, we stabilize the zero-phonon transition frequency against environmental fluctuations. This protocol reduces the zero-phonon fluorescence intensity noise by a factor of 22 by correcting for environmental noise with a bandwidth of 191 Hz, limited by the experimental collection efficiency. The associated sub-Hz fluctuations in the zero-phonon central frequency are reduced by a factor of 7. This technique provides a means of stabilizing the quantum dot emission frequency without requiring access to the zero-phonon emission.

  12. Ultra-sharp plasmonic resonances from monopole optical nanoantenna phased arrays

    SciTech Connect

    Li, Shi-Qiang; Bruce Buchholz, D.; Zhou, Wei; Ketterson, John B.; Ocola, Leonidas E.; Sakoda, Kazuaki; Chang, Robert P. H.

    2014-06-09

    Diffractively coupled plasmonic resonances possess both ultra-sharp linewidths and giant electric field enhancement around plasmonic nanostructures. They can be applied to create a new generation of sensors, detectors, and nano-optical devices. However, all current designs require stringent index-matching at the resonance condition that limits their applicability. Here, we propose and demonstrate that it is possible to relieve the index-matching requirement and to induce ultra-sharp plasmon resonances in an ordered vertically aligned optical nano-antenna phased array by transforming a dipole resonance to a monopole resonance with a mirror plane. Due to the mirror image effect, the monopole resonance not only retained the dipole features but also enhanced them. The engineered resonances strongly suppressed the radiative decay channel, resulting in a four-order of magnitude enhancement in local electric field and a Q-factor greater than 200.

  13. Ultra-sharp plasmonic resonances from monopole optical nanoantenna phased arrays

    NASA Astrophysics Data System (ADS)

    Li, Shi-Qiang; Zhou, Wei; Bruce Buchholz, D.; Ketterson, John B.; Ocola, Leonidas E.; Sakoda, Kazuaki; Chang, Robert P. H.

    2014-06-01

    Diffractively coupled plasmonic resonances possess both ultra-sharp linewidths and giant electric field enhancement around plasmonic nanostructures. They can be applied to create a new generation of sensors, detectors, and nano-optical devices. However, all current designs require stringent index-matching at the resonance condition that limits their applicability. Here, we propose and demonstrate that it is possible to relieve the index-matching requirement and to induce ultra-sharp plasmon resonances in an ordered vertically aligned optical nano-antenna phased array by transforming a dipole resonance to a monopole resonance with a mirror plane. Due to the mirror image effect, the monopole resonance not only retained the dipole features but also enhanced them. The engineered resonances strongly suppressed the radiative decay channel, resulting in a four-order of magnitude enhancement in local electric field and a Q-factor greater than 200.

  14. Electrons and Phonons in Semiconductor Multilayers

    NASA Astrophysics Data System (ADS)

    Ridley, B. K.

    2014-08-01

    Introduction; 1. Simple models of the electron-phonon interaction; 2. Quantum confinement of carriers; 3. Quasicontinuum theory of lattice vibrations; 4. Bulk vibratory modes in an isotropic continuum; 5. Optical modes in a quantum well; 6. Superlattice modes; 7. Optical modes in various structures; 8. Electron-phonon interaction in a quantum well; 9. Other scattering mechanisms; 10. Quantum screening; 11. The electron distribution function; 12. Spin relaxation; 13. Electrons and phonons in the Wurtzite lattice; 14. Nitride heterostructures; 15. Terahertz sources; References; Index.

  15. Optically Pumped Nuclear Magnetic Resonance in the Quantum Hall Regimes

    NASA Astrophysics Data System (ADS)

    Barrett, S. E.; Tycko, R.; Dabbagh, G.; Pfeiffer, L. N.; West, K. W.

    1996-03-01

    Optical pumping enables the direct detection of the nuclear magnetic resonance signal of ^71Ga nuclei located in an electron doped GaAs quantum well.footnote S. E. Barrett et al., Phys. Rev. Lett. 72, 1368 (1994) Using this technique, measurements of the Knight shiftfootnote S. E. Barrett et al., Phys. Rev. Lett. 74, 5112 (1995) and spin-lattice relaxation timefootnote R. Tycko et al., Science 268, 1460 (1995) have been carried out in the Quantum Hall regimes. It is clear from these measurements that probing the electronic spin degree of freedom can lead to new insights about the effect of interactions on the many-body ground state and low-lying excited states of these systems. For example, the Knight shift measurements provided the first experimental support for the recent theoretical predictionsfootnote S. L. Sondhi et al., Phys. Rev. B 47, 16419 (1993); H. A. Fertig et al., Phys. Rev. B 50, 11018 (1994) that the charged excitations of the ν = 1 ground state are novel spin textures called skyrmions. The current status of this picture will be discussed.

  16. Optically Pumped Nuclear Magnetic Resonance in the Quantum Hall Regimes

    NASA Astrophysics Data System (ADS)

    Barrett, S. E.; Khandelwal, P.; Kuzma, N. N.; Pfeiffer, L. N.; West, K. W.

    1997-03-01

    Optical pumping enables the direct detection of the nuclear magnetic resonance signal of ^71Ga nuclei located in an electron doped GaAs quantum well.footnote S. E. Barrett et al., Phys. Rev. Lett. 72, 1368 (1994) Using this technique, measurements of the Knight shift (K_S)footnote S. E. Barrett et al., Phys. Rev. Lett. 74, 5112 (1995) and spin-lattice relaxation time (T_1)footnote R. Tycko et al., Science 268, 1460 (1995) have been carried out in the Quantum Hall regimes. This talk will focus on our latest measurements of KS and T1 near Landau level filling ν=1, which extend our earlier results to higher magnetic fields (B=12 Tesla) and lower temperatures (T < 1 Kelvin). We will compare these results to the theoretical predictionsfootnote S. L. Sondhi et al., Phys. Rev. B 47, 16419 (1993); H. A. Fertig et al., Phys. Rev. B 50, 11018 (1994) that the charged excitations of the ν = 1 ground state are novel spin textures called skyrmions. The current status of this picture will be discussed.

  17. Deterministic phase engineering for optical Fano resonances with arbitrary lineshape and frequencies.

    PubMed

    Lin, Jiao; Huang, Lujun; Yu, Yiling; He, Sailing; Cao, Linyou

    2015-07-27

    We present an approach of deterministic phase engineering that can enable the rational design of optical Fano resonances with arbitrarily pre-specified lineshapes. Unlike all the approaches previously used to design optical Fano resonances, which fall short of designing the resonances with arbitrary lineshapes because of the lack of information for the optical phases involved, we develop our approach by capitalizing on unambiguous knowledge for the phase of optical modes. Optical Fano resonances arise from the interference of photons interacting with two optical modes with substantially different quality factors. We find that the phase difference of the two modes involved in optical Fano resonances is determined by the eigenfrequency difference of the modes. This allows us to deterministically engineer the phase by tuning the eigenfrequency, which may be very straightforward. We use dielectric grating structures as an example to illustrate the notion of deterministic engineering for the design of optical Fano resonances with arbitrarily pre-specified symmetry, linewidth, and wavelengths. PMID:26367578

  18. Phononic crystals and elastodynamics: Some relevant points

    SciTech Connect

    Aravantinos-Zafiris, N.; Sigalas, M. M.; Kafesaki, M.; Economou, E. N.

    2014-12-15

    In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation) with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.

  19. Engineering a resonant nanocoating for an optical refractive index sensor

    NASA Astrophysics Data System (ADS)

    Bialiayeu, A.; Ianoul, A.; Albert, J.

    2014-03-01

    We proposing to boost the performance of refractive index sensors based on the tilted fiber Bragg grating (TFBG) structure by resonant coupling of small spherical nanoparticles to the TFBG resonances. The optimal choice of nanoparticle parameters is discussed.

  20. Lasing from active optomechanical resonators

    PubMed Central

    Czerniuk, T.; Brüggemann, C.; Tepper, J.; Brodbeck, S.; Schneider, C.; Kamp, M.; Höfling, S.; Glavin, B. A.; Yakovlev, D. R.; Akimov, A. V.; Bayer, M.

    2014-01-01

    Planar microcavities with distributed Bragg reflectors (DBRs) host, besides confined optical modes, also mechanical resonances due to stop bands in the phonon dispersion relation of the DBRs. These resonances have frequencies in the 10- to 100-GHz range, depending on the resonator’s optical wavelength, with quality factors exceeding 1,000. The interaction of photons and phonons in such optomechanical systems can be drastically enhanced, opening a new route towards the manipulation of light. Here we implemented active semiconducting layers into the microcavity to obtain a vertical-cavity surface-emitting laser (VCSEL). Thereby, three resonant excitations—photons, phonons and electrons—can interact strongly with each other providing modulation of the VCSEL laser emission: a picosecond strain pulse injected into the VCSEL excites long-living mechanical resonances therein. As a result, modulation of the lasing intensity at frequencies up to 40 GHz is observed. From these findings, prospective applications of active optomechanical resonators integrated into nanophotonic circuits may emerge. PMID:25008784

  1. Intermolecular electron transfer from intramolecular excitation and coherent acoustic phonon generation in a hydrogen-bonded charge-transfer solid.

    PubMed

    Rury, Aaron S; Sorenson, Shayne; Dawlaty, Jahan M

    2016-03-14

    Organic materials that produce coherent lattice phonon excitations in response to external stimuli may provide next generation solutions in a wide range of applications. However, for these materials to lead to functional devices in technology, a full understanding of the possible driving forces of coherent lattice phonon generation must be attained. To facilitate the achievement of this goal, we have undertaken an optical spectroscopic study of an organic charge-transfer material formed from the ubiquitous reduction-oxidation pair hydroquinone and p-benzoquinone. Upon pumping this material, known as quinhydrone, on its intermolecular charge transfer resonance as well as an intramolecular resonance of p-benzoquinone, we find sub-cm(-1) oscillations whose dispersion with probe energy resembles that of a coherent acoustic phonon that we argue is coherently excited following changes in the electron density of quinhydrone. Using the dynamical information from these ultrafast pump-probe measurements, we find that the fastest process we can resolve does not change whether we pump quinhydrone at either energy. Electron-phonon coupling from both ultrafast coherent vibrational and steady-state resonance Raman spectroscopies allows us to determine that intramolecular electronic excitation of p-benzoquinone also drives the electron transfer process in quinhydrone. These results demonstrate the wide range of electronic excitations of the parent of molecules found in many functional organic materials that can drive coherent lattice phonon excitations useful for applications in electronics, photonics, and information technology. PMID:26979698

  2. Intermolecular electron transfer from intramolecular excitation and coherent acoustic phonon generation in a hydrogen-bonded charge-transfer solid

    NASA Astrophysics Data System (ADS)

    Rury, Aaron S.; Sorenson, Shayne; Dawlaty, Jahan M.

    2016-03-01

    Organic materials that produce coherent lattice phonon excitations in response to external stimuli may provide next generation solutions in a wide range of applications. However, for these materials to lead to functional devices in technology, a full understanding of the possible driving forces of coherent lattice phonon generation must be attained. To facilitate the achievement of this goal, we have undertaken an optical spectroscopic study of an organic charge-transfer material formed from the ubiquitous reduction-oxidation pair hydroquinone and p-benzoquinone. Upon pumping this material, known as quinhydrone, on its intermolecular charge transfer resonance as well as an intramolecular resonance of p-benzoquinone, we find sub-cm-1 oscillations whose dispersion with probe energy resembles that of a coherent acoustic phonon that we argue is coherently excited following changes in the electron density of quinhydrone. Using the dynamical information from these ultrafast pump-probe measurements, we find that the fastest process we can resolve does not change whether we pump quinhydrone at either energy. Electron-phonon coupling from both ultrafast coherent vibrational and steady-state resonance Raman spectroscopies allows us to determine that intramolecular electronic excitation of p-benzoquinone also drives the electron transfer process in quinhydrone. These results demonstrate the wide range of electronic excitations of the parent of molecules found in many functional organic materials that can drive coherent lattice phonon excitations useful for applications in electronics, photonics, and information technology.

  3. Athermalization of resonant optical devices via thermo-mechanical feedback

    DOEpatents

    Rakich, Peter; Nielson, Gregory N.; Lentine, Anthony L.

    2016-01-19

    A passively athermal photonic system including a photonic circuit having a substrate and an optical cavity defined on the substrate, and passive temperature-responsive provisions for inducing strain in the optical cavity of the photonic circuit to compensate for a thermo-optic effect resulting from a temperature change in the optical cavity of the photonic circuit. Also disclosed is a method of passively compensating for a temperature dependent thermo-optic effect resulting on an optical cavity of a photonic circuit including the step of passively inducing strain in the optical cavity as a function of a temperature change of the optical cavity thereby producing an elasto-optic effect in the optical cavity to compensate for the thermo-optic effect resulting on an optical cavity due to the temperature change.

  4. Cascaded Magneto-Optical Ring Resonator Structures for Tunable Faraday Rotation and Reduced Isolator Footprint

    NASA Astrophysics Data System (ADS)

    Cengiz Onbasli, Mehmet; Hu, Juejun; Bi, Lei; Dionne, Gerald F.; Ross, Caroline A.

    2012-02-01

    On-chip optical isolators are indispensible components of integrated optics, and can be modified to enable four-port and multi-port circulators and modulators. We have implemented an on-chip optical isolator by placing a racetrack resonator next to a single mode waveguide and coating half of the resonator with a uniformly magnetized magneto-optical film, which breaks the time-reversal symmetry of light propagation and provides different refractive indices and phase shifts for forward and backward propagating waves. At every pass, the optical mode inside the resonator accumulates Faraday rotation in addition to phase shift due to propagation. The transmission from the output port of the waveguide has a Lorentzian dip due to the resonance peak of the resonator. Light can only propagate in the clockwise direction inside the resonator. Here we model how cascading multiple ring resonators can increase the overall quality factor of the isolator and narrow the resonance linewidth, due to the longer photon lifetime inside the cavity. As a result of better control of Faraday rotation, the isolation ratio is enhanced and the device footprint is reduced with respect to Mach-Zehnder waveguide isolators.

  5. Measurements of depth dependent modification of optical constants arising from H+ implantation in n-type 4H-SiC using coherent acoustic phonons

    NASA Astrophysics Data System (ADS)

    Baydin, Andrey; Krzyzanowska, Halina; Dhanunjaya, M.; Rao, S. V. S. Nageswara; Davidson, Jimmy L.; Feldman, Leonard C.; Tolk, Norman H.

    Silicon carbide (SiC) is an ideal material for new electronics, such as high power/high temperature devices, and a candidate for advanced optical applications such as room temperature spintronics and quantum computing. Both types of applications may require the control of defects created by ion bombardment. In this work, we examine depth dependent modification of optical constants of 4H-SiC due to hydrogen implantation at 180keV and low doses ranging from 1014 to 1016 cm-2probed by coherent acoustic phonon (CAP) spectroscopy. For our studies, we used Si-face 10 μm epilayers of n-type 4H-SiC grown by CVD on 4H-SiC substrate. A comprehensive analysis of the reference and implanted spectra shows a strong dependence of 4H-SiC complex refractive index shape versus depth on the H+ fluence. We extract the complex refractive index as a function of depth and ion beam dose. Our results demonstrate that the implantation-modified refractive index is distributed over a greater depth range than Monte Carlo calculation predictions of the implantation induced structural damage. These studies provide insight into the application of hydrogen ion implantation to the fabrication of SiC-based photonic and optoelectronic devices. Work is supported by ARO under Contract No. W911NF-14-1-0290.

  6. Three-photon-absorption resonance for all-optical atomic clocks

    SciTech Connect

    Zibrov, Sergei; Novikova, Irina; Phillips, David F.; Taichenachev, Aleksei V.; Yudin, Valeriy I.; Walsworth, Ronald L.; Zibrov, Alexander S.

    2005-07-15

    We report an experimental study of an all-optical three-photon-absorption resonance (known as an 'N resonance') and discuss its potential application as an alternative to atomic clocks based on coherent population trapping. We present measurements of the N-resonance contrast, width and light shift for the D{sub 1} line of {sup 87}Rb with varying buffer gases, and find good agreement with an analytical model of this resonance. The results suggest that N resonances are promising for atomic clock applications.

  7. High-Q lithium niobate microdisk resonators on a chip for efficient electro-optic modulation.

    PubMed

    Wang, Jie; Bo, Fang; Wan, Shuai; Li, Wuxia; Gao, Feng; Li, Junjie; Zhang, Guoquan; Xu, Jingjun

    2015-09-01

    Lithium niobate (LN) microdisk resonators on a LN-silica-LN chip were fabricated using only conventional semiconductor fabrication processes. The quality factor of the LN resonator with a 39.6-μm radius and a 0.5-μm thickness is up to 1.19 × 10(6), which doubles the record of the quality factor 4.84 × 10(5) of LN resonators produced by microfabrication methods allowing batch production. Electro-optic modulation with an effective resonance-frequency tuning rate of 3.0 GHz/V was demonstrated in the fabricated LN microdisk resonator. PMID:26368411

  8. Sub-natural width resonances in Cs vapor confined in micrometric thickness optical cell

    NASA Astrophysics Data System (ADS)

    Cartaleva, S.; Krasteva, A.; Sargsyan, A.; Sarkisyan, D.; Slavov, D.; Vartanyan, T.

    2013-03-01

    We present here the behavior of Electromagnetically Induced Transparency (EIT), Velocity Selective Optical Pumping (VSOP) resonances and Velocity Selective Excitation (VSE) resonances observed in Cs vapor confined in а micrometric optical cell (MC) with thickness L = 6λ, λ = 852nm. For comparison of behavior of VSE resonance another conventional optical cell with thickness L=2.5 cm is used. Cells are irradiated in orthogonal to their windows directions by probe beam scanned on the Fg = 4 → Fe= 3, 4, 5 set of transitions and pump beam fixed at the Fg = 3 → Fe = 4 transition, on the D2 line of Cs. The enhanced absorption (fluorescence) narrow VSOP resonance at the closed transition transforms into reduced absorption (fluorescence) one with small increase of atomic concentration or light intensity. A striking difference appears between the VSE resonance broadening in L = 6λ and conventional L = 2.5cm cells.

  9. Ultrasensitive mass sensing with nonlinear optics in a doubly clamped suspended carbon nanotube resonator

    SciTech Connect

    Chen, Hua-Jun; Zhu, Ka-Di

    2013-12-07

    Nanomechanical resonator makes itself as an ideal system for ultrasensitive mass sensing due to its ultralow mass and high vibrational frequency. The mass sensing principle is due to the linear relationship of the frequency-shift and mass-variation. In this work, we will propose a nonlinear optical mass sensor based on a doubly clamped suspended carbon nanotube resonator in all-optical domain. The masses of external particles (such as nitric oxide molecules) landing onto the surface of carbon nanotube can be determined directly and accurately via using the nonlinear optical spectroscopy. This mass sensing proposed here may provide a nonlinear optical measurement technique in quantum measurements and environmental science.

  10. Magneto-optic transmittance modulation observed in a hybrid graphene-split ring resonator terahertz metasurface

    NASA Astrophysics Data System (ADS)

    Zanotto, Simone; Lange, Christoph; Maag, Thomas; Pitanti, Alessandro; Miseikis, Vaidotas; Coletti, Camilla; Degl'Innocenti, Riccardo; Baldacci, Lorenzo; Huber, Rupert; Tredicucci, Alessandro

    2015-09-01

    By placing a material in close vicinity of a resonant optical element, its intrinsic optical response can be tuned, possibly to a wide extent. Here, we show that a graphene monolayer, spaced a few tenths of nanometers from a split ring resonator metasurface, exhibits a magneto-optical response which is strongly influenced by the presence of the metasurface itself. This hybrid system holds promises in view of thin optical modulators, polarization rotators, and nonreciprocal devices, in the technologically relevant terahertz spectral range. Moreover, it could be chosen as the playground for investigating the cavity electrodynamics of Dirac fermions in the quantum regime.

  11. INEX modeling of the Boeing ring optical resonator free-electron laser

    SciTech Connect

    Goldstein, J.C.; Tokar, R.L.; McVey, B.D.; Elliott, C.J. ); Dowell, D.H.; Laucks, M.L.; Lowrey, A.R. )

    1990-01-01

    We present new results from the integrated numerical model of the accelerator/beam transport system and ring optical resonator of the Boeing free-electron laser experiment. Modifications of the electron-beam transport have been included in a previously developed PARMELA model and are shown to reduce dramatically emittance growth in the 180{degree} bend. The new numerically generated electron beam is used in the 3-D FEL simulation code FELEX to calculate expected laser characteristics with the ring optical resonator and the 5-m untapered THUNDER wiggler. Gain, extraction efficiency, and optical power are compared with experimental data. Performance sensitivity to optical cavity misalignments is studied.

  12. Piezoelectric resonance calorimetry of nonlinear-optical crystals under laser irradiation

    NASA Astrophysics Data System (ADS)

    Ryabushkin, Oleg A.; Konyashkin, Aleksey V.; Myasnikov, Daniil V.; Tyrtyshnyy, Valentin A.; Vershinin, Oleg I.

    2013-09-01

    Novel method is proposed for determination of nonlinear-optical crystal both heat transfer and optical absorption coefficients by measuring kinetics of the laser-irradiated crystal temperature-dependent piezoelectric resonance frequency. When laser radiation propagates through the crystal its temperature evaluation with time is directly determined from crystal piezoelectric resonance frequency shift, which is precisely measured by analyzing crystal response to the applied ac electric voltage. Heat transfer and optical absorption coefficients are obtained using measured characteristic time of crystal laser heating kinetics by solving nonstationary heat conduction equation. Experiments were performed with nonlinear-optical α-quartz, lithium triborate (LBO) and periodically poled lithium niobate (PPLN) crystals.

  13. Magneto-optic transmittance modulation observed in a hybrid graphene–split ring resonator terahertz metasurface

    SciTech Connect

    Zanotto, Simone; Pitanti, Alessandro; Lange, Christoph; Maag, Thomas; Huber, Rupert; Miseikis, Vaidotas; Coletti, Camilla; Degl'Innocenti, Riccardo; Baldacci, Lorenzo; Tredicucci, Alessandro

    2015-09-21

    By placing a material in close vicinity of a resonant optical element, its intrinsic optical response can be tuned, possibly to a wide extent. Here, we show that a graphene monolayer, spaced a few tenths of nanometers from a split ring resonator metasurface, exhibits a magneto-optical response which is strongly influenced by the presence of the metasurface itself. This hybrid system holds promises in view of thin optical modulators, polarization rotators, and nonreciprocal devices, in the technologically relevant terahertz spectral range. Moreover, it could be chosen as the playground for investigating the cavity electrodynamics of Dirac fermions in the quantum regime.

  14. Surface plasmon optical antennae in the infrared region with high resonant efficiency and frequency selectivity.

    PubMed

    Ueno, Kosei; Sun, Quan; Mino, Masahiro; Itoh, Takumi; Oshikiri, Tomoya; Misawa, Hiroaki

    2016-08-01

    Infrared light has received attention for sensor applications, including fingerprint spectroscopy, in the bioengineering and security fields. Surface plasmon physics enables the operation of a light harvesting optical antenna. Gold nanochains exhibit localized surface plasmon resonance (LSPR) in the infrared region with high frequency selectivity. However, a feasible design for optical antennae with a higher resonant efficiency and frequency selectivity as a function of structural design and periodicity is still unknown. In the present study, we investigated the relationship between the resonant efficiency and frequency selectivity as a function of the structural design of gold nanochains and explored structural periodicity for obtaining highly frequency-selective optical antennae. An optical antenna design with higher resonant efficiency is proposed on the basis of its efficient interaction with non-polarized light. PMID:27505741

  15. Laterally vibrating resonator based elasto-optic modulation in aluminum nitride

    NASA Astrophysics Data System (ADS)

    Ghosh, Siddhartha; Piazza, Gianluca

    2016-06-01

    An integrated strain-based optical modulator driven by a piezoelectric laterally vibrating resonator is demonstrated. The composite structure consists of an acoustic Lamb wave resonator, in which a photonic racetrack resonator is internally embedded to enable overlap of the guided optical mode with the induced strain field. Both types of resonators are defined in an aluminum nitride (AlN) thin film, which rests upon a layer of silicon dioxide in order to simultaneously define optical waveguides, and the structure is released from a silicon substrate. Lateral vibrations produced by the acoustic resonator are transferred through a partially etched layer of AlN, producing a change in the effective index of the guided wave through the interaction of the strain components with the AlN elasto-optic (p) coefficients. Optical modulation through the elasto-optic effect is demonstrated at electromechanically actuated frequencies of 173 MHz and 843 MHz. This device geometry further enables the development of MEMS-based optical modulators in addition to studying elasto-optic interactions in suspended piezoelectric thin films.

  16. Optically Pumped Nuclear Magnetic Resonance in the Quantum Hall Regimes

    NASA Astrophysics Data System (ADS)

    Barrett, Sean E.

    1998-03-01

    Optical pumping enables the direct detection of the nuclear magnetic resonance signal of ^71Ga nuclei located in an electron doped GaAs quantum well.footnote S. E. Barrett et al., Phys. Rev. Lett. 72, 1368 (1994) This OPNMR technique was previously used to measure the Knight shift (K_S)footnote S. E. Barrett et al., Phys. Rev. Lett. 74, 5112 (1995) and spin-lattice relaxation time (T_1)footnote R. Tycko et al., Science 268, 1460 (1995) near Landau level filling ν=1, which provided the first experimental support for the theoretical predictionsfootnote S. L. Sondhi et al., Phys. Rev. B 47, 16419 (1993); H. A. Fertig et al., Phys. Rev. B 50, 11018 (1994) that the charged excitations of the ν = 1 ground state are novel spin textures called skyrmions. We have recently demonstrated that OPNMR is possible in fields up to B=12 Tesla, and temperatures down to T= 0.3 K, making it a viable new probe of the Fractional Quantum Hall Regime. In this talk we will present our latest OPNMR measurements near Landau level filling ν=1/3, which include the first direct measurement of the electron spin polarization at ν=1/3. The spin polarization drops as the filling factor is varied away from ν=1/3, indicating that the quasiparticles and quasiholes are not fully spin-polarized. We will also show how the NMR lineshape away from ν=1/3 changes dramatically at low temperatures, which is due to slowing of the electron dynamics, and a reduction in the motional narrowing of the NMR line. The current understanding of these results will be discussed.

  17. Optical Control of Magnetic Feshbach Resonances by Closed-Channel Electromagnetically Induced Transparency

    NASA Astrophysics Data System (ADS)

    Jagannathan, A.; Arunkumar, N.; Joseph, J. A.; Thomas, J. E.

    2016-02-01

    We control magnetic Feshbach resonances in an optically trapped mixture of the two lowest hyperfine states of a 6Li Fermi gas, using two optical fields to create a dark state in the closed molecular channel. In the experiments, the narrow Feshbach resonance is tuned by up to 3 G. For the broad resonance, the spontaneous lifetime is increased to 0.4 s at the dark-state resonance, compared to 0.5 ms for single-field tuning. We present a new model of light-induced loss spectra, employing continuum-dressed basis states, which agrees in shape and magnitude with loss measurements for both broad and narrow resonances. Using this model, we predict the trade-off between tunability and loss for the broad resonance in 6Li, showing that our two-field method substantially reduces the two-body loss rate compared to single-field methods for the same tuning range.

  18. Continuous spectrum of modes for optical micro-sphere resonators

    NASA Astrophysics Data System (ADS)

    Nooramin, Amir Saman; Shahabadi, Mahmoud

    2016-09-01

    This paper presents an improved modal analysis for the spherical dielectric resonator. This is commonly carried out by assuming an outgoing spherical Hankel function for the region surrounding the dielectric sphere. It will be shown that this assumption is incomplete and cannot lead to the entire spectrum of resonance frequencies. Following an analytical formulation, we prove that, like cylindrical resonators, the only choice for the outer region of the dielectric sphere can be a proper linear combination of an inward and an outward traveling wave. Starting from this formulation, we determine the complete spectrum of the resonance frequencies and the associated mode fields. In this analysis, the continuous spectrum of resonance frequencies is introduced and the properties of radiation modes are studied in detail. The proposed analytical formulation is thereafter employed to calculate the quality factor of the resonator due to radiation and dielectric loss.

  19. Optical field emission from resonant gold nanorods driven by femtosecond mid-infrared pulses

    SciTech Connect

    Kusa, F.; Echternkamp, K. E.; Herink, G.; Ropers, C.; Ashihara, S.

    2015-07-15

    We demonstrate strong-field photoelectron emission from gold nanorods driven by femtosecond mid-infrared optical pulses. The maximum photoelectron yield is reached at the localized surface plasmon resonance, indicating that the photoemission is governed by the resonantly-enhanced optical near-field. The wavelength- and field-dependent photoemission yield allows for a noninvasive determination of local field enhancements, and we obtain intensity enhancement factors close to 1300, in good agreement with finite-difference time domain computations.

  20. Optical-Fiber-Illuminated Response of a Superconducting Microwave Resonator Below 1 K

    NASA Astrophysics Data System (ADS)

    Voigt, Kristen; Hertzberg, J. B.; Dutta, S. K.; Hoffman, J. E.; Grover, J. A.; Lee, J.; Solano, P.; Budoyo, R. P.; Ballard, C.; Anderson, J. R.; Lobb, C. J.; Rolston, S. L.; Wellstood, F. C.

    As a step towards building a hybrid quantum system that couples superconducting elements to neutral atoms trapped on a tapered optical nanofiber, we have studied how the presence of the fiber dielectric and light scattered from a fiber affect the response of a translatable thin-film lumped-element superconducting Al microwave resonator that is cooled to 15 mK. The resonator has a resonance frequency of about 6 GHz, a quality factor Q 2 x 105, and is mounted inside a 3D Al superconducting cavity. An optical fiber is tapered to a 60 um diameter and passes through two small holes in the 3D cavity such that it sits near the resonator. The 3D cavity is mounted on an x-z piezo-translation stage that allows us to change the relative position of the thin-film resonator and fiber. When the resonator is brought closer to the fiber, the resonance frequency decreases slightly due to the presence of the fiber dielectric. When 200 uW of 780 nm light is sent through the fiber, about 100 pW/mm is Rayleigh-scattered from the fiber. This causes a position-dependent illumination of the resonator, affecting its resonance frequency and Q. We compare our results to a model of the resonator response that includes the generation, diffusion, and recombination of quasiparticles in the resonator and find that the frequency response allows us to track the position of the fiber to within 10 um.