Science.gov

Sample records for short-lived neutron-deficient nuclei

  1. Photodissociation of neutron deficient nuclei

    NASA Astrophysics Data System (ADS)

    Sonnabend, K.; Babilon, M.; Hasper, J.; Müller, S.; Zarza, M.; Zilges, A.

    2006-03-01

    The knowledge of the cross sections for photodissociation reactions like e.g. (γ, n) of neutron deficient nuclei is of crucial interest for network calculations predicting the abundances of the so-called p nuclei. However, only single cross sections have been measured up to now, i.e., one has to rely nearly fully on theoretical predictions. While the cross sections of stable isotopes are accessible by experiments using real photons, the bulk of the involved reactions starts from unstable nuclei. Coulomb dissociation (CD) experiments in inverse kinematics might be a key to expand the experimental database for p-process network calculations. The approach to test the accuracy of the CD method is explained.

  2. The Onset of Deformation in Neutron-Deficient At Nuclei

    SciTech Connect

    Smith, M.B.; Chapman, R.; Cocks, J.F.C.; Dorvaux, O.; Helariutta, K.; Jones, P.M.; Julin, R.; Juutinen, S.; Kankaanpaa, H.; Kettunen, H.; Kuusiniemi, P.; Le Coz, Y.; Leino, M.; Middleton, D.J.; Muikku, M.; Nieminen, P.; Rahkila, P.; Savelius, A.; Spohr, K.-M.

    1999-12-31

    Excited states in the {sup 197}At nucleus have been identified for the first time using the recoil-decay-tagging technique. The excitation energy of these states is found to be consistent with the systematics of neutron-deficient At nuclei and with calculations indicating that the nucleus may be deformed in its ground state. A more recent experiment, to study states in {sup 195}At, is discussed.

  3. The onset of deformation in neutron-deficient At nuclei

    SciTech Connect

    Smith, M. B.; Chapman, R.; Middleton, D. J.; Spohr, K.-M.; Cocks, J. F. C.; Dorvaux, O.; Helariutta, K.; Jones, P. M.; Julin, R.; Juutinen, S.; Kankaanpaeae, H.; Kettunen, H.; Kuusiniemi, P.; Leino, M.; Muikku, M.; Nieminen, P.; Rahkila, P.; Savelius, A.; Coz, Y. Le

    1999-11-16

    Excited states in the {sup 197}At nucleus have been identified for the first time using the recoil-decay-tagging technique. The excitation energy of these states is found to be consistent with the systematics of neutron-deficient. At nuclei and with calculations indicating that the nucleus may be deformed in its ground state. A more recent experiment, to study states in {sup 195}At, is discussed.

  4. Probe of Triple Shape Coexistence In Neutron Deficient Polonium Nuclei

    SciTech Connect

    Wiseman, D. R.; Page, R. D.; Darby, I. G.; Andreyev, A. N.; Eeckhaudt, S.; Grahn, T.; Greenlees, P. T.; Jones, P.; Julin, R.; Juutinen, S.; Kettunen, H.; Leino, M.; Leppaenen, A.-P.; Nyman, M.; Pakarinen, J.; Rahkila, P.; Saren, J.; Scholey, C.; Uusitalo, J.; Sandzelius, M.

    2006-04-26

    {gamma}-ray transitions in the neutron deficient 190,197Po nuclei have been identified. The yrast band of 190Po has been extended up to a spin and parity of 14+ and is found to display similar systematic behaviour to isotones 186Hg and 188Pb above the 4+ level, thus confirming its prolate nature. In 197Po the band built upon the 13/2+ isomer has been extended up to a spin and parity of 33/2+, while the non-yrast side-band has been observed for the first time. The behaviour of 197Po is found to be similar to that of the nearby even-mass isotopes, which is consistent with the model in which the i13/2 neutron is weakly coupled to the states in the even-even core.

  5. First demonstration of electron scattering using a novel target developed for short-lived nuclei.

    PubMed

    Suda, T; Wakasugi, M; Emoto, T; Ishii, K; Ito, S; Kurita, K; Kuwajima, A; Noda, A; Shirai, T; Tamae, T; Tongu, H; Wang, S; Yano, Y

    2009-03-13

    We carried out a demonstrative electron scattering experiment using a novel ion-trap target exclusively developed for short-lived highly unstable nuclei. Using stable 133Cs ion as a target, this experiment completely mimicked electron scattering off short-lived nuclei. Achieving a luminosity higher than 10;{26} cm;{-2} s;{-1} with around only 10;{6} trapped ions on the electron beam, the angular distribution of elastic scattering was successfully measured. This experiment clearly demonstrates that electron scattering off rarely produced short-lived nuclei is practical with this target technique. PMID:19392108

  6. First Demonstration of Electron Scattering Using a Novel Target Developed for Short-Lived Nuclei

    SciTech Connect

    Suda, T.; Wakasugi, M.; Emoto, T.; Ito, S.; Wang, S.; Yano, Y.; Ishii, K.; Kurita, K.; Kuwajima, A.; Tamae, T.; Noda, A.; Shirai, T.; Tongu, H.

    2009-03-13

    We carried out a demonstrative electron scattering experiment using a novel ion-trap target exclusively developed for short-lived highly unstable nuclei. Using stable {sup 133}Cs ion as a target, this experiment completely mimicked electron scattering off short-lived nuclei. Achieving a luminosity higher than 10{sup 26} cm{sup -2} s{sup -1} with around only 10{sup 6} trapped ions on the electron beam, the angular distribution of elastic scattering was successfully measured. This experiment clearly demonstrates that electron scattering off rarely produced short-lived nuclei is practical with this target technique.

  7. Four-Quasiparticle High-K States in Neutron-Deficient Lead and Polonium Nuclei

    NASA Astrophysics Data System (ADS)

    Shi, Yue; Xu, Furong

    2012-06-01

    Configuration-constrained potential energy surface calculations have been performed to investigate four-quasiparticle high-K configurations in neutron-deficient lead and polonium isotopes. A good agreement between the calculations and the experimental data has been found for the excitation energy of the observed Kπ = 19- state in 188Pb. Several lowly excited high-K states are predicted, and the large oblate deformation and low energy indicate high-K isomerism in these nuclei.

  8. Probing collectivity in the vicinity of neutron deficient Pb nuclei

    SciTech Connect

    Grahn, T.; Page, R. D.; Petts, A.; Dewald, A.; Jolie, J.; Melon, B.; Pissulla, Th.; Hornillos, M. B. Gomez; Greenlees, P. T.; Jones, P.; Julin, R.; Juutinen, S.; Ketelhut, S.; Leino, M.; Nyman, M.; Rahkila, P.; Saren, J.; Scholey, C.; Sorri, J.; Uusitalo, J.

    2008-05-12

    A series of recoil distance Doppler-shift lifetime measurements have been carried out to probe collectivity and configuration mixing of different shapes in the vicinity of neutron mid-shell Pb nuclei. Lifetime measurements of {sup 186}Pb and {sup 194}Po, the first ever utilizing the recoil-decay tagging method, probed the collectivity of coexisting prolate and oblate shapes in this region. Futher lifetime measurements of excited states in {sup 180}Hg, {sup 182}Hg and {sup 196}Po have been carried out.

  9. Projected Shell Model Study of Yrast States of Neutron-Deficient Odd-Mass Pr Nuclei

    SciTech Connect

    Ibanes, A.; Ortiz, Mark E; Velazquez, V.; Galindo-Uribarri, Alfredo {nmn}; Hess, P. O.; Sun, Y.

    2011-01-01

    A wide variety of modern instruments allow us to study neutron-deficient nuclei in the A = 130 mass region. Highly deformed nuclei have been found in this region, providing opportunities to study the deformed rotational bands. The description of the 125,127,129,131,133Pr isotopes with the projected shell model is presented in this paper. Good agreement between theory and experiment is obtained and some characteristics are discussed, including the dynamic moment of inertia J (2), kinetic moment of inertia J (1), the crossing of rotational bands, and backbending effects.

  10. Projected shell model study of yrast states of neutron-deficient odd-mass Pr nuclei

    SciTech Connect

    Ibanez-Sandoval, A.; Ortiz, M. E.; Velazquez, V.; Galindo-Uribarri, A.; Hess, P. O.; Sun, Y.

    2011-03-15

    A wide variety of modern instruments allow us to study neutron-deficient nuclei in the A=130 mass region. Highly deformed nuclei have been found in this region, providing opportunities to study the deformed rotational bands. The description of the {sup 125,127,129,131,133}Pr isotopes with the projected shell model is presented in this paper. Good agreement between theory and experiment is obtained and some characteristics are discussed, including the dynamic moment of inertia J{sup (2)}, kinetic moment of inertia J{sup (1)}, the crossing of rotational bands, and backbending effects.

  11. Projected shell model study of yrast states of neutron-deficient odd-mass Pr nuclei

    NASA Astrophysics Data System (ADS)

    Ibáñez-Sandoval, A.; Ortiz, M. E.; Velázquez, V.; Galindo-Uribarri, A.; Hess, P. O.; Sun, Y.

    2011-03-01

    A wide variety of modern instruments allow us to study neutron-deficient nuclei in the A=130 mass region. Highly deformed nuclei have been found in this region, providing opportunities to study the deformed rotational bands. The description of the Pr125,127,129,131,133 isotopes with the projected shell model is presented in this paper. Good agreement between theory and experiment is obtained and some characteristics are discussed, including the dynamic moment of inertia J(2), kinetic moment of inertia J(1), the crossing of rotational bands, and backbending effects.

  12. Spectroscopy of low-lying states in neutron-deficient astatine and francium nuclei

    SciTech Connect

    Jakobsson, U. Cederwall, B.; Uusitalo, J.; Auranen, K.; Badran, H.; Cox, D. M.; Grahn, T.; Greenlees, P. T.; Julin, R.; Juutinen, S.; Herzáň, A.; Konki, J.; Leino, M.; Mallaburn, M.; Pakarinen, J.; Papadakis, P.; Partanen, J.; Rahkila, P.; Sandzelius, M.; Sarén, J.; and others

    2015-10-15

    Low-lying states in neutron-deficient astatine and francium nuclei have been studied by means of in-beam and delayed spectroscopy. The 13/2{sup +} state has been observed in francium nuclei with a similar down-sloping trend as in neighbouring astatine and bismuth isotopes, as a function of decreasing neutron number. A systematic trend can also now be seen for the 1/2{sup +} state both in astatine and francium nuclei, where the level energy decreases steeply as a function of neutron number when moving further away from the neutron shell closure. This trend is very similar between astatine nuclei and their francium isotones. Moreover, shape coexistence has been observed between the 13/2{sup +} state and the spherical 9/2{sup −} ground state in {sup 203}Fr and {sup 205}Fr.

  13. Spectroscopy of low-lying states in neutron-deficient astatine and francium nuclei

    NASA Astrophysics Data System (ADS)

    Jakobsson, U.; Uusitalo, J.; Auranen, K.; Badran, H.; Cederwall, B.; Cox, D. M.; Grahn, T.; Greenlees, P. T.; Julin, R.; Juutinen, S.; HerzáÅ, A.; Konki, J.; Leino, M.; Mallaburn, M.; Pakarinen, J.; Papadakis, P.; Partanen, J.; Rahkila, P.; Sandzelius, M.; Sarén, J.; Scholey, C.; Sorri, J.; Stolze, S.

    2015-10-01

    Low-lying states in neutron-deficient astatine and francium nuclei have been studied by means of in-beam and delayed spectroscopy. The 13/2+ state has been observed in francium nuclei with a similar down-sloping trend as in neighbouring astatine and bismuth isotopes, as a function of decreasing neutron number. A systematic trend can also now be seen for the 1/2+ state both in astatine and francium nuclei, where the level energy decreases steeply as a function of neutron number when moving further away from the neutron shell closure. This trend is very similar between astatine nuclei and their francium isotones. Moreover, shape coexistence has been observed between the 13/2+ state and the spherical 9/2- ground state in 203Fr and 205Fr.

  14. Theoretical study of evaporation cross sections in the synthesis of very neutron-deficient nuclei

    SciTech Connect

    Wang Chengbin; Zhang Jinjuan; Ren, Z. Z.

    2011-07-15

    The synthesis of rare-earth neutron-deficient nuclei with large Z/N ratio {approx_equal}0.88 is studied within the framework of the standard statistical model. The fusion cross sections are calculated on the basis of the nuclear reaction video model. The deexcitation process is calculated with the help of the statistical code alice. It is found that the excitation functions can be predicted using a few exited experimental data by carefully choosing the input parameters in the statistical model. The results obtained show that a satisfactory description of the experimental evaporation cross sections requires a great reduction in the theoretical fission barriers.

  15. Chiral Symmetry and Signature Splitting in Odd-Odd Neutron deficient Pr Nuclei

    NASA Astrophysics Data System (ADS)

    Fetea, Mirela; Nikolova, Veronika; Crider, Benjamin

    2004-10-01

    Over the past few years, sufficient data have been accumulated to enable a meaningful study of the systematic trends in nuclei far from stability. While general characteristics seen in experiments are understood by various mean-field nuclear models, there are key features that are not fully explained. Of particular interest are the chiral symmetry (chiral bands) and signature splitting/inversion phenomena. We report on our investigation on the association of signature inversion in an odd-odd band of two quasiparticles pointed along different axes with the formation of chiral twin bands, and understanding systematic chiral symmetry and signature splitting/inversion features within the framework of particle rotor model for neutron deficient Pr nuclei. This work was supported by the NSF Grant No. PHY 0204811 and U.S. Research Corporation Grant No. CC5494.

  16. Failure of the gross theory of beta decay in neutron deficient nuclei

    SciTech Connect

    Firestone, R. B.; Schwengner, R.; Zuber, K.

    2015-05-28

    The neutron deficient isotopes 117-121Xe, 117-124Cs, and 122-124Ba were produced by a beam of 28Si from the LBNL SuperHILAC on a target of natMo. The isotopes were mass separated and their beta decay schemes were measured with a Total Absorption Spectrometer (TAS). The beta strengths derived from these data decreased dramatically to levels above ≈1 MeV for the even-even decays; 3–4 MeV for even-Z, odd-N decays; 4–5 MeV for the odd-Z, even-N decays; and 7–8 MeV for the odd-Z, odd-N decays. The decreasing strength to higher excitation energies in the daughters contradicts the predictions of the Gross Theory of Beta Decay. The integrated beta strengths are instead found to be consistent with shell model predictions where the single-particle beta strengths are divided amoung many low-lying levels. The experimental beta strengths determined here have been used calculate the half-lives of 143 neutron deficient nuclei with Z=51–64 to a precision of 20% with respect to the measured values.

  17. Failure of the gross theory of beta decay in neutron deficient nuclei

    DOE PAGESBeta

    Firestone, R. B.; Schwengner, R.; Zuber, K.

    2015-05-28

    The neutron deficient isotopes 117-121Xe, 117-124Cs, and 122-124Ba were produced by a beam of 28Si from the LBNL SuperHILAC on a target of natMo. The isotopes were mass separated and their beta decay schemes were measured with a Total Absorption Spectrometer (TAS). The beta strengths derived from these data decreased dramatically to levels above ≈1 MeV for the even-even decays; 3–4 MeV for even-Z, odd-N decays; 4–5 MeV for the odd-Z, even-N decays; and 7–8 MeV for the odd-Z, odd-N decays. The decreasing strength to higher excitation energies in the daughters contradicts the predictions of the Gross Theory of Betamore » Decay. The integrated beta strengths are instead found to be consistent with shell model predictions where the single-particle beta strengths are divided amoung many low-lying levels. The experimental beta strengths determined here have been used calculate the half-lives of 143 neutron deficient nuclei with Z=51–64 to a precision of 20% with respect to the measured values.« less

  18. Mass Measurement of Short-lived Nuclei at HIRFL-CSR

    NASA Astrophysics Data System (ADS)

    Wang, M.; Xu, H. S.; Zhang, Y. H.; Tu, X. L.; Litvinov, Yu. A.

    2014-03-01

    Four campaigns of mass measurements for short-lived nuclei have been conducted using an isochronous mass spectrometry (IMS) technique at HIRFL-CSR(Cooler Storage Ring) in Lanzhou. The radioactive nuclei were produced by projectile fragmentation and injected into the experimental storage ring CSRe. Revolution times of the ions stored in the CSRe were measured from which masses of 78Kr, 58Ni, 86Kr and 112Sn fragments have been determined with a relative uncertainty of about 10-6-10-7. The experimental results are presented and their impacts on nucleosynthesis in the rp process and nuclear structure are discussed.

  19. In-beam spectroscopic studies of shape coexistence and collectivity in the neutron-deficient Z ≈ 82 nuclei

    NASA Astrophysics Data System (ADS)

    Julin, R.; Grahn, T.; Pakarinen, J.; Rahkila, P.

    2016-02-01

    In the present paper we focus on studies of shape coexistence in even-mass nuclei in the neutron-deficient Pb region. They are based on experiments carried out using tagging techniques in the Accelerator Laboratory of the University of Jyväskylä, Finland. Excited states in many of these nuclei can only be accessed via fusion-evaporation reactions employing high-intensity stable-ion beams. The key features in these experiments are high selectivity, clean spectra and instrumentation that enables high count rates. We review three spectroscopic highlights in this region.

  20. AGB stars as a source of short-lived radioactive nuclei in the solar nebula

    NASA Technical Reports Server (NTRS)

    Wasserburg, G. J.; Gallino, R.; Busso, M.; Raiteri, C. M.

    1993-01-01

    The purpose is to estimate the possible contribution of some short-lived nuclei to the early solar nebula from asymptotic giant branch (AGB) sources. Low mass (1 to 3 solar mass) AGB stars appear to provide a site for synthesis of the main s process component for solar system material with an exponential distribution of neutron irradiations varies as exp(-tau/tau(sub 0)) (where tau is the time integrated neutron flux with a mean neutron exposure tau(sub 0)) for solar abundances with tau(sub 0) = 0.28 mb(sup -1). Previous workers estimated the synthesis of key short-lived nuclei which might be produced in AGB stars. While these calculations exhibit the basic characteristics of nuclei production by neutron exposure, there is need for a self-consistent calculation that follows AGB evolution and takes into account the net production from a star and dilution with the cloud medium. Many of the general approaches and the conclusions arrived at were presented earlier by Cameron. The production of nuclei for a star of 1.5 solar mass during the thermal pulsing of the AGB phase was evaluated. Calculations were done for a series of thermal pulses with tau(sub 0) = 0.12 and 0.28 mb(sup -1). These pulses involve s nucleosynthesis in the burning shell at the base of the He zone followed by the ignition of the H burning shell at the top of the He zone. After about 10-15 cycles the abundances of the various nuclei in the He zone become constant. Computations of the abundances of all nuclei in the He zone were made following Gallino. The mass of the solar nebula was considered to consist of some initial material of approximately solar composition plus some contributions from AGB stars. The ratios of the masses required from the AGB He burning zone to the ISM necessary to produce the observed value of Pd-107/Pd-108 in the early solar system were calculated and this dilution factor was applied to all other relevant nuclei.

  1. Developments in precison mass measurements of short-lived r-process nuclei with CARIBU

    NASA Astrophysics Data System (ADS)

    Marley, S. T.; Aprahamian, A.; Mumpower, M.; Nystrom, A.; Paul, N.; Siegl, K.; Strauss, S.; Surman, R.; Clark, J. A.; Perez Galvan, A.; Savard, G.; Morgan, G.; Orford, R.

    2013-10-01

    The confluence of new radioactive beam facilities and modern precision mass spectrometry techniques now make it possible to measure masses of many neutron-rich nuclei important to nuclear structure and astrophysics. A recent mass sensitivity study (S. Brett et al., Eur. Phys. J., A 48, 184 (2012)) identified the nuclear masses that are the most influential to the final rapid-neutron capture process abundance distributions under various astrophysical scenarios. This work motivated a campaign of precision mass measurements using the Canadian Penning Trap (CPT) installed at the Californium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory. In order to measure the weakest and most short-lived (t1/2 < 150 ms) of these influential nuclei, a series of upgrades to the CARIBU and CPT systems have been developed. The implementation of these upgrades, the r-process mass measurements, and the status of CARIBU facilty will be discussed. This work performed under the auspices of NSERC, Canada, appl. # 216974, the U.S. DOE, Office of Nuclear Physics, under contracts DE-AC02-06CH11357, DE-FG02-91ER-40609, DE-FG02-98ER41086, & DE-AC52-07NA27344, and NSF Grants PHY08-22648 and PHY-106819.

  2. Distributions of Short-lived Radioactive Nuclei Produced by Young Embedded Star Clusters

    NASA Astrophysics Data System (ADS)

    Adams, Fred C.; Fatuzzo, Marco; Holden, Lisa

    2014-07-01

    Most star formation in the Galaxy takes place in clusters, where the most massive members can affect the properties of other constituent solar systems. This paper considers how clusters influence star formation and forming planetary systems through nuclear enrichment from supernova explosions, where massive stars deliver short-lived radioactive nuclei (SLRs) to their local environment. The decay of these nuclei leads to both heating and ionization, and thereby affects disk evolution, disk chemistry, and the accompanying process of planet formation. Nuclear enrichment can take place on two spatial scales: (1) within the cluster itself (l ~ 1 pc), the SLRs are delivered to the circumstellar disks associated with other cluster members. (2) On the next larger scale (l ~ 2-10 pc), SLRs are injected into the background molecular cloud; these nuclei provide heating and ionization to nearby star-forming regions and to the next generation of disks. For the first scenario, we construct the expected distributions of radioactive enrichment levels provided by embedded clusters. Clusters can account for the SLR mass fractions inferred for the early Solar Nebula, but typical SLR abundances are lower by a factor of ~10. For the second scenario, we find that distributed enrichment of SLRs in molecular clouds leads to comparable abundances. For both the direct and distributed enrichment processes, the masses of 26Al and 60Fe delivered to individual circumstellar disks typically fall in the range 10-100 pM ⊙ (where 1 pM ⊙ = 10-12 M ⊙). The corresponding ionization rate due to SLRs typically falls in the range ζSLR ~ 1-5 × 10-19 s-1. This ionization rate is smaller than that due to cosmic rays, ζCR ~ 10-17 s-1, but will be important in regions where cosmic rays are attenuated (e.g., disk mid-planes).

  3. Sizes and shapes of short-lived nuclei via laser spectroscopy. Progress report, May 1, 1980-January 31, 1981

    SciTech Connect

    Lewis, D.A.

    1981-02-01

    The first stage of the program to study the sizes and shapes of short-lived nuclei through their atomic hyperfine structure is to develop a movable laser spectroscopy system. This system is now almost complete and is described in this report along with plans for measurements at Argonne National Laboratory and Brookhaven National Laboratory.

  4. Mass measurements of the neutron-deficient 41Ti, 45Cr, 49Fe, and 53Ni nuclides: first test of the isobaric multiplet mass equation in f p-shell nuclei.

    PubMed

    Zhang, Y H; Xu, H S; Litvinov, Yu A; Tu, X L; Yan, X L; Typel, S; Blaum, K; Wang, M; Zhou, X H; Sun, Y; Brown, B A; Yuan, Y J; Xia, J W; Yang, J C; Audi, G; Chen, X C; Jia, G B; Hu, Z G; Ma, X W; Mao, R S; Mei, B; Shuai, P; Sun, Z Y; Wang, S T; Xiao, G Q; Xu, X; Yamaguchi, T; Yamaguchi, Y; Zang, Y D; Zhao, H W; Zhao, T C; Zhang, W; Zhan, W L

    2012-09-01

    Isochronous mass spectrometry has been applied to neutron-deficient 58Ni projectile fragments at the HIRFL-CSR facility in Lanzhou, China. Masses of a series of short-lived T(z)=-3/2 nuclides including 41Ti, 45Cr, 49Fe, and 53Ni have been measured with a precision of 20-40 keV. The new data enable us to test for the first time the isobaric multiplet mass equation (IMME) in fp-shell nuclei. We observe that the IMME is inconsistent with the generally accepted quadratic form for the A=53, T=3/2 quartet. We perform full space shell model calculations and compare them with the new experimental results. PMID:23005283

  5. Multi-quasiparticle excitation: Extending shape coexistence in A{approx}190 neutron-deficient nuclei

    SciTech Connect

    Shi Yue; Liu, H. L.; Xu, F. R.; Walker, P. M.

    2010-10-15

    Multi-quasiparticle high-K states in neutron-deficient mercury, lead, and polonium isotopes have been investigated systematically by means of configuration-constrained potential-energy-surface calculations. An abundance of high-K states is predicted with both prolate and oblate shapes, which extends the shape coexistence of the mass region. Well-deformed shapes provide good conditions for the formation of isomers, as exemplified in {sup 188}Pb. Of particular interest is the prediction of low-lying 10{sup -} states in polonium isotopes, which indicate long-lived isomers.

  6. Multi-quasiparticle excitation: Extending shape coexistence in A~190 neutron-deficient nuclei

    NASA Astrophysics Data System (ADS)

    Shi, Yue; Xu, F. R.; Liu, H. L.; Walker, P. M.

    2010-10-01

    Multi-quasiparticle high-K states in neutron-deficient mercury, lead, and polonium isotopes have been investigated systematically by means of configuration-constrained potential-energy-surface calculations. An abundance of high-K states is predicted with both prolate and oblate shapes, which extends the shape coexistence of the mass region. Well-deformed shapes provide good conditions for the formation of isomers, as exemplified in Pb188. Of particular interest is the prediction of low-lying 10- states in polonium isotopes, which indicate long-lived isomers.

  7. Distributions of short-lived radioactive nuclei produced by young embedded star clusters

    SciTech Connect

    Adams, Fred C.; Fatuzzo, Marco; Holden, Lisa

    2014-07-01

    Most star formation in the Galaxy takes place in clusters, where the most massive members can affect the properties of other constituent solar systems. This paper considers how clusters influence star formation and forming planetary systems through nuclear enrichment from supernova explosions, where massive stars deliver short-lived radioactive nuclei (SLRs) to their local environment. The decay of these nuclei leads to both heating and ionization, and thereby affects disk evolution, disk chemistry, and the accompanying process of planet formation. Nuclear enrichment can take place on two spatial scales: (1) within the cluster itself (ℓ ∼ 1 pc), the SLRs are delivered to the circumstellar disks associated with other cluster members. (2) On the next larger scale (ℓ ∼ 2-10 pc), SLRs are injected into the background molecular cloud; these nuclei provide heating and ionization to nearby star-forming regions and to the next generation of disks. For the first scenario, we construct the expected distributions of radioactive enrichment levels provided by embedded clusters. Clusters can account for the SLR mass fractions inferred for the early Solar Nebula, but typical SLR abundances are lower by a factor of ∼10. For the second scenario, we find that distributed enrichment of SLRs in molecular clouds leads to comparable abundances. For both the direct and distributed enrichment processes, the masses of {sup 26}Al and {sup 60}Fe delivered to individual circumstellar disks typically fall in the range 10-100 pM {sub ☉} (where 1 pM {sub ☉} = 10{sup –12} M {sub ☉}). The corresponding ionization rate due to SLRs typically falls in the range ζ{sub SLR} ∼ 1-5 × 10{sup –19} s{sup –1}. This ionization rate is smaller than that due to cosmic rays, ζ{sub CR} ∼ 10{sup –17} s{sup –1}, but will be important in regions where cosmic rays are attenuated (e.g., disk mid-planes).

  8. Deformation of the very neutron-deficient rare-earth nuclei produced with the SPIRAL 76Kr radioactive beam and studied with EXOGAM + DIAMANT

    NASA Astrophysics Data System (ADS)

    Redon, N.; Prévost, A.; Guinet, D.; Lautesse, Ph.; Meyer, M.; Rossé, B.; Stézowski, O.; Nolan, P. J.; Andreoiu, C.; Boston, A. J.; Descovich, M.; Evans, A. O.; Gros, S.; Norman, J.; Page, R. D.; Paul, E. S.; Rainovski, G.; Sampson, J.; de France, G.; Casandjian, J. M.; Theisen, Ch.; Scheurer, J. N.; Nyakó, B. M.; Gál, J.; Kalinka, G.; Molnár, J.; Dombrádi, Zs.; Timár, J.; Zolnai, L.; Juhász, K.; Astier, A.; Deloncle, I.; Porquet, M. G.; Wadsworth, R.; Raddon, P.; Lee, Y.; Wilkinson, A.; Joshi, P.; Simpson, J.; Appelbe, D.; Joss, D.; Lemmon, R.; Smith, J.; Cullen, D.; Brondi, A.; La Rana, G.; Moro, R.; Vardacci, E.; Girod, M.

    2004-02-01

    The structure of the very neutron-deficient rare-earth nuclei has been investigated in the first experiment with the EXOGAM gamma array coupled to the DIAMANT light charged particle detector using radioactive beam of 76Kr delivered by the SPIRAL facility. Very neutron-deficient Pr, Nd and Pm isotopes have been populated at rather high spin by the reaction 76Kr + 58Ni at a beam energy of 328 MeV. We report here the first results of this experiment.

  9. Deformation of the very neutron-deficient rare-earth nuclei produced with the SPIRAL 76Kr radioactive beam and studied with EXOGAM + DIAMANT

    SciTech Connect

    Redon, N.; Guinet, D.; Lautesse, Ph.; Meyer, M.; Rosse, B.; Stezowski, O.; France, G. de; Casandjian, J. M.

    2004-02-27

    The structure of the very neutron-deficient rare-earth nuclei has been investigated in the first experiment with the EXOGAM gamma array coupled to the DIAMANT light charged particle detector using radioactive beam of 76Kr delivered by the SPIRAL facility. Very neutron-deficient Pr, Nd and Pm isotopes have been populated at rather high spin by the reaction 76Kr + 58Ni at a beam energy of 328 MeV. We report here the first results of this experiment.

  10. Electron-capture delayed fission properties of neutron-deficient einsteinium nuclei

    SciTech Connect

    Shaughnessy, Dawn A.

    2000-01-05

    Electron-capture delayed fission (ECDF) properties of neutron-deficient einsteinium isotopes were investigated using a combination of chemical separations and on-line radiation detection methods. {sup 242}Es was produced via the {sup 233}U({sup 14}N,5n){sup 242}Es reaction at a beam energy of 87 MeV (on target) in the lab system, and was found to decay with a half-life of 11 {+-} 3 seconds. The ECDF of {sup 242}Es showed a highly asymmetric mass distribution with an average pre-neutron emission total kinetic energy (TKE) of 183 {+-} 18 MeV. The probability of delayed fission (P{sub DF}) was measured to be 0.006 {+-} 0.002. In conjunction with this experiment, the excitation functions of the {sup 233}U({sup 14}N,xn){sup 247{minus}x}Es and {sup 233}U({sup 15}N,xn){sup 248{minus}x}Es reactions were measured for {sup 243}Es, {sup 244}Es and {sup 245}Es at projectile energies between 80 MeV and 100 MeV.

  11. Structural evolution of the Z=52-62 neutron-deficient nuclei in the interacting boson approximation framework

    SciTech Connect

    Pascu, S.; Cata-Danil, Gh.; Zamfir, N. V.; Marginean, N.

    2010-05-15

    The interacting boson approximation (IBA) is employed in the present article to follow the structural evolution of the neutron-deficient nuclei from the Z=52-62 region. The IBA model parameters are determined to reproduce the properties of the low-lying positive parity excitations for a wide range of even-even collective nuclei. The parameters aim to describe simultaneously the existing electromagnetic data (energy levels, transition matrix elements, etc.) and hadronic ones (two-nucleon transfer intensities). It is shown that a simple Hamiltonian with only two terms is not adequate to describe the properties across this region. It is found that the octupole term plays an important role in reproducing the properties of the 2{sub g}amma{sup +} and 0{sub 2}{sup +} states, as well as in the description of the two-neutron transfer intensities patterns. A mapping of these parameters in the IBA symmetry triangle allows the comparison of representative trajectories for different isotopic chains.

  12. Identification of isomeric states in the N=73 neutron-deficient nuclei 132Pr and 130La

    NASA Astrophysics Data System (ADS)

    Taylor, M. J.; Alharshan, G. A.; Cullen, D. M.; Procter, M. G.; Lumley, N. M.; Grahn, T.; Greenlees, P. T.; Hauschild, K.; Herzan, A.; Jakobsson, U.; Jones, P.; Julin, R.; Juutinen, S.; Ketelhut, S.; Leino, M.; Lopez-Martens, A.; Nieminen, P.; Partanen, J.; Peura, P.; Rahkila, P.; Rinta-Antila, S.; Ruotsalainen, P.; Sandzelius, M.; Sarén, J.; Scholey, C.; Sorri, J.; Stolze, S.; Uusitalo, J.; Xu, F. R.; Bai, Z. J.

    2012-10-01

    Decays from isomeric states in the neutron-deficient N=73 nuclei 132Pr and 130La have been observed for the first time. Half-lives of 486(70) ns and 2.46(4) μs were measured for two isomeric states in 132Pr. The decay from the 486 ns (8-) isomer has been interpreted as a hindered E1 transition from the bandhead state of the excited πh11/2⊗νg7/2 configuration. The decay from the 2.5 μs (8+) isomer is consistent with the Weisskopf estimate for a low-energy E2 transition. An analogous 0.74(3) μs decay from an (8+) isomer in the neighboring isotone 130La has also been observed which similarly can be explained if the transition has E2 character. The Weisskopf interpretation for the isomer hindrance is strengthened by the lack of evidence for shape or K isomerism due to the γ-soft shapes predicted by configuration-constrained potential-energy-surface calculations.

  13. New Developments for Isochronous Mass Measurements of Short-Lived Nuclei

    SciTech Connect

    Knoebel, R.; Litvinov, S. A.; Boutin, D.; Chen, L.; Geissel, H.; Litvinov, Yu. A.; Scheidenberger, C.; Winckler, N.; Sun, B.; Beckert, K.; Beller, P.; Bosch, F.; Brandau, C.; Dimopoulou, C.; Dolinskii, A.; Kozhuharov, C.; Mazzocco, M.; Montes, F.; Muenzenberg, G.; Nociforo, C.

    2007-02-26

    The combination of the in-flight separator FRS and the storage-ring ESR at GSI offers unique possibilities for high accuracy mass and lifetime measurements of bare and few-electron fragments. Operating the ESR in the isochronous mode allows for measurements of revolution frequencies of stored ions without cooling. Isochronous Mass Spectrometry (IMS) can be applied to fragments with half-lives as short as several tens of microseconds. Newly developed magnetic rigidity tagging increases the resolving power of IMS to about 500000. IMS can be used to measure masses of nuclei with rates even lower than one ion per day, a property also needed for the purpose of the ILIMA project at the future facility FAIR.

  14. Spatial and Time Coincidence Detection of the Decay Chain of Short-Lived Radioactive Nuclei

    SciTech Connect

    Granja, Carlos; Jakubek, Jan; Platkevic, Michal; Pospisil, Stanislav

    2010-08-04

    The quantum counting position sensitive pixel detector Timepix with per-pixel energy and time resolution enables to detect radioactive ions and register the consecutive decay chain by simultaneous position-and time-correlation. This spatial and timing coincidence technique in the same sensor is demonstrated by the registration of the decay chain {sup 8}He{yields}{sup {beta} 8}Li and {sup 8}Li{yields}{sup {beta}-} {sup 8}Be{yields}{alpha}+{alpha} and by the measurement of the {beta} decay half-lives. Radioactive ions, selectively obtained from the Lohengrin fission fragment spectrometer installed at the High Flux Reactor of the ILL Grenoble, are delivered to the Timepix silicon sensor where decays of the implanted ions and daughter nuclei are registered and visualized. We measure decay lifetimes in the range {>=}{mu}s with precision limited just by counting statistics.

  15. Asymptotic Giant Branch stars as a source of short-lived radioactive nuclei in the solar nebula

    NASA Technical Reports Server (NTRS)

    Wasserburg, G. J.; Busso, M.; Gallino, R.; Raiteri, C. M.

    1994-01-01

    We carried out a theoretical evaluation of the contribution of Asymptotic Giant Branch (AGB) stars to some short-lived (10(exp 6) less than or equal to Tau-bar less than or equal to 2 x 10(exp 7) yr) isotopes in the Interstellar Medium (ISM) and in the early solar system using stellar model calculations for thermally pulsing evolutionary phases of low-mass stars. The yields of s-process nuclei in the convective He-shell for different neutron exposures tau(sub 0) were obtained, and AGB stars were shown to produce several radioactive nuclei (especially Pd-107, Pb-205, Fe-60, Zr-93, Tc-99, Cs-135, and Hf-182) in diferent amounts. Assuming either contamination of the solar nebula from a single AGB star or models for continuous injection and mixing from many stars into the ISM, we calculate the ratios of radioactive to stable nuclei at the epoch of the Sun's formation. The dilution factor between the AGB ejecta and the early solar system matter is obtained by matching the observed Pd-107/Pd-108 and depends on the value of tau(sub 0). It is found that small masses M(sub He) of He-shell material (10(exp -4)-10(exp -7) solar mass) enriched in s-process nuclei are sufficient to contaminate 1 solar mass of the ISM to produce the Pd-107 found in the early solar system. Predictions are made for all of the other radioactive isotopes. The optimal model to explain several observed radioactive species at different states of the proto-solar nebula involves a single AGB star with a low neutron exposure (tau(sub 0) = 0.03 mbarn(sup -1)) which contaminated the cloud with a dilution factor of M(sub He)/solar mass approximately 1.5 x 10(exp -4). This will also contribute newly synthesized stable s-process nuclei in the amount of approximately 10(exp -4) of their abundances already present in the proto-solar cloud. Variations in the degree of homogenization (approximately 30%) of the injected material may account for some of the small general isotopic anomalies found in meteorites. It is

  16. Tentative study of nuclear charge radii for neutron-deficient nuclei around the Z = 82 shell from experimental α decay data

    NASA Astrophysics Data System (ADS)

    Qian, Yibin; Ren, Zhongzhou

    2016-01-01

    We tentatively investigate the root-mean-square (rms) nuclear charge radii of odd-A Po and Pb isotopes plus Tl isotopes, particularly concerning these difficultly-detected nuclei along with short lifetimes, via various data on α decay. Within the density-dependent cluster model, the density distributions of studied daughter nuclei are determined by exactly reproducing the corresponding experimental α decay half-lives, which leads the final results of nuclear charge radii. In addition, our recently proposed formula deducing the charge radii is extended to this study for comparison. Whether it concerns the ground or isomeric state of target nuclei, the extracted nuclear charge radii are found to be in good agreement with the measured values. Sequential predictions on the rms charge radii are subsequently made for these neutron-deficient nuclei and especially for the rarely detected Bi isotopic chain, which are expected to be useful for future measurements. Moreover, the variety of α-preformation factors is analyzed in the scheme of valence nucleon number to pursue the further improvement of the model. This may be considered as an effective effort to obtain the charge radii of ground and even low-lying excited states for exotic nuclei near the proton-dripline.

  17. β+/EC decay rates of deformed neutron-deficient nuclei in the deformed QRPA with realistic interactions

    NASA Astrophysics Data System (ADS)

    Ni, Dongdong; Ren, Zhongzhou

    2015-05-01

    The weak-decay (β+ and EC) rates of neutron-deficient Kr, Sr, Zr, and Mo isotopes are investigated within the deformed quasiparticle random-phase approximation with realistic nucleon-nucleon interactions. The particle-particle and particle-hole channels of residual interactions are handled in large single-particle model spaces, based on the Brückner G-matrix with charge-dependent Bonn nucleon-nucleon forces. Contributions from allowed Gamow-Teller and Fermi transitions as well as first-forbidden transitions are calculated. The calculated half-lives show good agreement with the experimental data over a wide range of magnitude, from 10-2 to 107 s. Moreover, predictions of β-decay half-lives are made for some extremely proton-rich isotopes, which could be useful for future experiments.

  18. Design Study for a Multi-Reflection Time-of-Flight Mass Spectrograph for Very Short Lived Nuclei

    NASA Astrophysics Data System (ADS)

    Yoon, Jin Woo; Park, Young-Ho; Im, Kang-Bin; Kim, Gi Dong; Kim, Yong Kyun

    The multi-reflection time-of-flight mass spectrometer (MR-TOF-MS) has been designed for the high precision mass measurement system in RAON accelerator facility, which will be constructed in Korea. Mirror-electrode potentials were numerically optimized by Nelder-Mead algorithm. The temporal spread and the mass-resolving power were calculated for the 132Sn+ ions with an energy spread of 20 eV and an emittance of 3 π mm mrad; the mass resolving power over 105 was achieved. MR-TOF-MS will be used for the isobar separation and the mass measurement for very short-lived isotopes.

  19. A high-speed target-rotation system (taro) for the study of short-lived nuclei

    NASA Astrophysics Data System (ADS)

    Miyatake, H.; Hama, H.; Kamiya, T.; Yoshii, M.; Shinozuka, T.; Fujioka, M.

    1986-05-01

    We describe the design and performance of a high-speed target-rotation system for the study of nuclei far from stability, by which targets can be transported to the detector position in 60 ms after irradiation (90° rotation). The rotor movement and the cyclotron beam pulsing, as well as the data acquisition, are controlled by a microcomputer. Using this device 54Co (T {1}/{2} = 193 ms) and 58Cu (T {1}/{2} = 3.2 s) were observed in a test experiment with a transport efficiency of 71 and 98%, respectively (180° rotation).

  20. [Short-lived disorders].

    PubMed

    Artigas-Pallares, Josep

    2012-02-29

    Over the years, most of the mental disorders that are dealt with in everyday clinical practice have changed not only their names but also their conceptualisation. Furthermore, as some disorders disappear or are forgotten, others come into being. Seen from a historical perspective and unlike many of the diseases included within classical medicine, it can be stated that one of the basic characteristics of mental disorders is their short-lived presence in the scientific literature. In this study we analyse the causes underlying the transitory nature of mental disorders. The disappearance of a disorder or the modification of how it is conceptualised may be linked to several different motives. Sometimes they may be due to an evolution of the construct, as a result of new findings. On other occasions the disorder falls into disuse owing to the weakness of the theoretical construct or the clinical research upholding it. Lastly, because the Diagnostic and Statistical Manual of Mental Disorders and the International Classification of Diseases require updates that incorporate new contributions and correct faults in the current model, they give rise to new denominations and definitions in mental disorders. This article analyses these three situations and offers an illustrative example in each case. PMID:22374762

  1. Shape Coexistence in Neutron Deficient Po Nuclei

    SciTech Connect

    Helariutta, K.; Cocks, J.F.C.; Enqvist, T.; Greenlees, P.T.; Jones, P.; Julin, R.; Juutinen, S.; Jamsen, P.; Kankaanpaa, H.; Kettunen, H.; Kuiusiniemi, P.; Leino, M.; Muikkui, M.; Piiparinen, M.; Rahkila, P.; Savelius, A.; Trzaska, W.H.; Tormanen, S.; Uusitalo, J.; Allatt, R.G.; Butler, P.A.; Page, R.D.; Kapusta, M.

    1999-12-31

    The excited levels in {sup 192-195}Po have been studied using the recoil-decay tagging method. New levels have been identified. The data are in accordance with the scheme of the coexisting spherical and deformed intruder structures crossing each other with N<112.

  2. Shape coexistence in neutron deficient Po nuclei

    SciTech Connect

    Helariutta, K.; Cocks, J. F. C.; Enqvist, T.; Greenlees, P. T.; Jones, P.; Julin, R.; Juutinen, S.; Jaemsen, P.; Kankaanpaeae, H.; Kettunen, H.; Kuusiniemi, P.; Leino, M.; Muikku, M.; Piiparinen, M.; Rahkila, P.; Savelius, A.; Trzaska, W. H.; Toermaenen, S.; Uusitalo, J.; Allatt, R. G.

    1999-11-16

    The excited levels in {sup 192-195}Po have been studied using the recoil-decay tagging method. New levels have been identified. The data are in accordance with the scheme of the coexisting spherical and deformed intruder structures crossing each other with N<112.

  3. Efficiency and rate capability studies of the time-of-flight detector for isochronous mass measurements of stored short-lived nuclei with the FRS-ESR facility

    NASA Astrophysics Data System (ADS)

    Kuzminchuk-Feuerstein, Natalia; Fabian, Benjamin; Diwisch, Marcel; Plaß, Wolfgang R.; Geissel, Hans; Ayet San Andrés, Samuel; Dickel, Timo; Knöbel, Ronja; Scheidenberger, Christoph; Sun, Baohua; Weick, Helmut

    2016-06-01

    A time-of-flight (TOF) detector is used for Isochronous Mass Spectrometry (IMS) with the projectile fragment separator FRS and the heavy-ion storage ring ESR. Exotic nuclei are spatially separated in flight with the FRS at about 70% of the speed of light and are injected into the ESR. The revolution times of the stored ions circulating in the ESR are measured with a thin transmission foil detector. When the ions penetrate the thin detector foil, secondary electrons (SEs) are emitted from the surface and provide the timing information in combination with microchannel plate (MCP) detectors. The isochronous transport of the SEs is performed by perpendicular superimposed electric and magnetic fields. The detection efficiency and the rate capability of the TOF detector have been studied in simulations and experiments. As a result the performance of the TOF detector has been improved substantially: (i) The SE collection efficiency was doubled by use of an optimized set of electric and magnetic field values; now SEs from almost the full area of the foil are transmitted to the MCP detectors. (ii) The rate capability of the TOF detector was improved by a factor of four by the use of MCPs with 5 μm pore size. (iii) With these MCPs and a carbon foil with a reduced thickness of 10 μg/cm2 the number of recorded revolutions in the ESR has been increased by nearly a factor of 10. The number of recorded revolutions determine the precision of the IMS experiments. Heavy-ion measurements were performed with neon ions at 322 MeV/u and uranium fission fragments at about 370 MeV/u. In addition, measurements with an alpha source were performed in the laboratory with a duplicate of the TOF detector.

  4. Short-Lived Climate Pollution

    NASA Astrophysics Data System (ADS)

    Pierrehumbert, R. T.

    2014-05-01

    Although carbon dioxide emissions are by far the most important mediator of anthropogenic climate disruption, a number of shorter-lived substances with atmospheric lifetimes of under a few decades also contribute significantly to the radiative forcing that drives climate change. In recent years, the argument that early and aggressive mitigation of the emission of these substances or their precursors forms an essential part of any climate protection strategy has gained a considerable following. There is often an implication that such control can in some way make up for the current inaction on carbon dioxide emissions. The prime targets for mitigation, known collectively as short-lived climate pollution (SLCP), are methane, hydrofluo-rocarbons, black carbon, and ozone. A re-examination of the issues shows that the benefits of early SLCP mitigation have been greatly exaggerated, largely because of inadequacies in the methodologies used to compare the climate effects of short-lived substances with those of CO2, which causes nearly irreversible climate change persisting millennia after emissions cease. Eventual mitigation of SLCP can make a useful contribution to climate protection, but there is little to be gained by implementing SLCP mitigation before stringent carbon dioxide controls are in place and have caused annual emissions to approach zero. Any earlier implementation of SLCP mitigation that substitutes to any significant extent for carbon dioxide mitigation will lead to a climate irreversibly warmer than will a strategy with delayed SLCP mitigation. SLCP mitigation does not buy time for implementation of stringent controls on CO2 emissions.

  5. Photodisintegration studies on p-nuclei: the case of Mo and sm isotopes

    NASA Astrophysics Data System (ADS)

    Nair, C.; Junghans, A. R.; Erhard, M.; Bemmerer, D.; Beyer, R.; Crespo, P.; Grosse, E.; Fauth, M.; Kosev, K.; Rusev, G.; Schilling, K. D.; Schwengner, R.; Wagner, A.

    2008-01-01

    In explosive stellar environments like supernovae, the temperatures are high enough for the production of heavy neutron-deficient nuclei, the so-called p-nuclei. Up to now, the knowledge of the reaction rates of p-nuclei is based on theoretical parameterizations using statistical model calculations. At the bremsstrahlung facility of the superconducting electron accelerator ELBE of FZ Dresden Rossendorf, we aim to measure the photodisintegration rates of heavy nuclei experimentally. Photoactivation measurements on the astrophysically relevant p-nuclei 92Mo and 144Sm have been performed with bremsstrahlung end-point energies from 10.0 to 16.5 MeV. First experiments on the short-lived decays following the reaction 144Sm(γ,n) are carried out using a pneumatic delivery system for rapid transport of activated samples. The activation yields are compared with calculations using cross sections from recent Hauser Feshbach models.

  6. Experiment for synthesis of neutron-deficient protactinium isotopes

    NASA Astrophysics Data System (ADS)

    Yang, Huabin; Ma, Long; Zhang, Zhiyuan; Yu, Lin; Jia, Guobin; Huang, Minghui; Gan, Zaiguo; Huang, Tianheng; Li, Guangshun; Wu, Xiaolei; Fang, Yongde; Wang, Zhigang; Gao, Bingshui; Hua, Wei

    2014-10-01

    The complete fusion reaction 40Ca+175Lu was studied at a beam energy of 5.1 MeV u-1. Evaporation residues recoiled from the target were separated from the primary beam by the gas-filled recoil separator SHANS and then implanted into the focal plane detection system. Based on the energy-position-time correlation measurement, neutron-deficient nuclei 208-213Ac, 212Pa and 211Th produced in this reaction were identified. Previously reported decay properties of the ground state in 212Pa were confirmed and improved values of 5.1_{-1.7}^{+5.1} ms and 8.250(20) MeV for the half-life and α-particle energy of 212Pa were obtained. No correlated decay chain arising from 211Pa was observed and an upper limit for the cross section of 211Pa was estimated.

  7. β-decay properties of neutron-deficient Pt, Hg, and Pb isotopes

    SciTech Connect

    Sarriguren, P.; Boillos, J. M.; Moreno, O.; Moya de Guerra, E.

    2015-10-15

    Neutron-deficient isotopes in the lead region are well established examples of the shape coexistence phenomenon in nuclei. In this work, bulk and decay properties, including deformation energy curves, charge mean square radii, Gamow-Teller (GT) strength distributions, and β-decay half-lives, are studied in neutron-deficient Pt, Hg, and Pb isotopes. The nuclear structure involved is described microscopically from deformed quasiparticle random-phase approximation calculations with residual interactions in both particle-hole and particle-particle channels, performed on top of a self-consistent deformed quasiparticle Skyrme Hartree-Fock basis. The sensitivity to deformation of the GT strength distributions in those isotopes is proposed as an additional complementary signature of the nuclear shape. The β-decay half-lives resulting from the GT strength distributions are compared to experiment to demonstrate the ability of the method.

  8. First Use of High Charge States for Mass Measurements of Short-Lived Nuclides in a Penning Trap

    SciTech Connect

    Ettenauer, S.; Gallant, A. T.; Dilling, J.; Simon, M. C.; Chaudhuri, A.; Mane, E.; Delheij, P.; Pearson, M. R.; Brunner, T.; Chowdhury, U.; Simon, V. V.; Brodeur, M.; Andreoiu, C.; Audi, G.; Lopez-Urrutia, J. R. Crespo; Ullrich, J.; Gwinner, G.; Lapierre, A.; Lunney, D.; Ringle, R.

    2011-12-30

    Penning trap mass measurements of short-lived nuclides have been performed for the first time with highly charged ions, using the TITAN facility at TRIUMF. Compared to singly charged ions, this provides an improvement in experimental precision that scales with the charge state q. Neutron-deficient Rb isotopes have been charge bred in an electron beam ion trap to q=8-12+ prior to injection into the Penning trap. In combination with the Ramsey excitation scheme, this unique setup creating low energy, highly charged ions at a radioactive beam facility opens the door to unrivaled precision with gains of 1-2 orders of magnitude. The method is particularly suited for short-lived nuclides such as the superallowed {beta} emitter {sup 74}Rb (T{sub 1/2}=65 ms). The determination of its atomic mass and an improved Q{sub EC} value are presented.

  9. First use of high charge states for mass measurements of short-lived nuclides in a Penning trap.

    PubMed

    Ettenauer, S; Simon, M C; Gallant, A T; Brunner, T; Chowdhury, U; Simon, V V; Brodeur, M; Chaudhuri, A; Mané, E; Andreoiu, C; Audi, G; López-Urrutia, J R Crespo; Delheij, P; Gwinner, G; Lapierre, A; Lunney, D; Pearson, M R; Ringle, R; Ullrich, J; Dilling, J

    2011-12-30

    Penning trap mass measurements of short-lived nuclides have been performed for the first time with highly charged ions, using the TITAN facility at TRIUMF. Compared to singly charged ions, this provides an improvement in experimental precision that scales with the charge state q. Neutron-deficient Rb isotopes have been charge bred in an electron beam ion trap to q=8-12+ prior to injection into the Penning trap. In combination with the Ramsey excitation scheme, this unique setup creating low energy, highly charged ions at a radioactive beam facility opens the door to unrivaled precision with gains of 1-2 orders of magnitude. The method is particularly suited for short-lived nuclides such as the superallowed β emitter 74Rb (T(1/2)=65  ms). The determination of its atomic mass and an improved Q(EC) value are presented. PMID:22243307

  10. Skylab short-lived event alert program

    NASA Technical Reports Server (NTRS)

    Citron, R. A.

    1974-01-01

    During the three manned Skylab missions, the Center for Short-Lived Phenomena (CSLP) reported a total of 39 significant events to the Johnson Space Center (JSC) as part of the Skylab Short-Lived Event Alert Program. The telegraphed daily status reports included the names and locations of the events, the track number and revolution number during which the event could be observed, the time (GMT) to within plus or minus 2 sec when Skylab was closest to the event area, and the light condition (daylight or darkness) at that time and place. The messages sent to JSC during the Skylab 4 mission also included information pertaining to ground-truth studies and observations being conducted on the events. Photographic priorities were assigned for each event.

  11. Alchemy with short-lived radionuclides

    SciTech Connect

    Rubio, F.F.; Finn, R.D.; Gilson, A.J.

    1981-04-01

    A variety of short-lived radionuclides are produced and subsequently incorporated into radiopharmaceutical compounds in the radionuclide production program currently being conducted at the Cyclotron Facility of Mount Sinai Medical Center. The recovery of high specific activity oxygen-15 labelled water prepared by means of an inexpensive system operating in conjunction with an on-line radiogas target routinely utilized for oxygen-15 labelled carbon dioxide studies is currently receiving particular attention.

  12. β Decay in the Region of Neutron-deficient {sup 69,70,71}Kr

    SciTech Connect

    Rogers, A.M.; Giovinazzo, J.; Blank, B.; Canchel, G.; France, G. de; Grévy, S.; Oliveira Santos, F. de; Stefan, I.; Thomas, J.-C.

    2014-06-15

    Decay spectroscopy was performed for neutron-deficient nuclei ranging from zinc to krypton with isospin −3/2 ≤T{sub z}≤0. Measurements of correlated β-delayed protons allowed us to determine the isobaric analog states fed from the decay of {sup 65}Se and {sup 69}Kr, constraining the spin of the {sup 69}Kr ground state. Preliminary results regarding the half lives for the T{sub z}=−1 systems, relevant to the rapid proton capture (rp) process, are discussed.

  13. Low-lying excited states in the neutron-deficient isotopes 163Os and 165Os

    NASA Astrophysics Data System (ADS)

    Drummond, M. C.; Joss, D. T.; Page, R. D.; Simpson, J.; O'Donnell, D.; Andgren, K.; Bianco, L.; Cederwall, B.; Darby, I. G.; Eeckhaudt, S.; Gomez-Hornillos, M. B.; Grahn, T.; Greenlees, P. T.; Hadinia, B.; Jones, P. M.; Julin, R.; Juutinen, S.; Ketelhut, S.; Leppänen, A.-P.; Leino, M.; Nyman, M.; Pakarinen, J.; Rahkila, P.; Sandzelius, M.; Sapple, P. J.; Sarén, J.; Saygi, B.; Scholey, C.; Sorri, J.; Thomson, J.; Uusitalo, J.; Venhart, M.

    2013-05-01

    Excited states in the neutron-deficient isotopes 163Os and 165Os were identified using the JUROGAM and GREAT spectrometers in conjunction with the RITU gas-filled separator. The 163Os and 165Os nuclei were populated via the 106Cd(60Ni,3n) and 92Mo(78Kr,2p3n) reactions at bombarding energies of 270 MeV and 357 MeV, respectively. Gamma-ray emissions from these nuclei have been established unambiguously using the recoil-decay tagging technique and a coincidence analysis has allowed level schemes to be established. These results suggest that the yrast states are based upon negative-parity configurations originating from the νf7/2 and νh9/2 orbitals.

  14. Short-lived radioactivity and magma genesis.

    PubMed

    Gill, J; Condomines, M

    1992-09-01

    Short-lived decay products of uranium and thorium have half-lives and chemistries sensitive to the processes and time scales of magma genesis, including partial melting in the mantle and magmatic differentiation in the crust. Radioactive disequilibrium between (238)U, (230)Th, and (226)Ra is widespread in volcanic rocks. These disequilibria and the isotopic composition of thorium depend especially on the extent and rate of melting as well as the presence and composition of vapor during melting. The duration of mantle melting may be several hundred millennia, whereas ascent times are a few decades to thousands of years. Differentiation of most magmas commonly occurs within a few millennia, but felsic ones can be tens of millennia old upon eruption. PMID:17738278

  15. Beta delayed alpha emission from the neutron deficient rare earth isotopes {sup 152}Tm and {sup 150}Ho

    SciTech Connect

    Nacher, E.; Tain, J. L.; Rubio, B.; Algora, A.; Estevez Aguado, M. E.; Gadea, A.; Batist, L.; Briz, J. A.; Cano-Ott, D.; Doering, J.; Mukha, I.; Plettner, C.; Roeckl, E.; Gierlik, M.; Janas, Z.

    2011-11-30

    The study of beta-delayed proton emission is a well known method to aid the determination of the beta strength distribution in nuclei far from the stability line. At the neutron deficient side of the nuclear chart the process of proton or alpha emission from excited states is energetically allowed when one goes far enough from stability. However, beta-delayed alphas have seldom been measured for nuclei heavier than A = 20. Here we present a study of the beta-delayed alpha-particle emission from {sup 152}Tm and {sup 150}Ho and their importance in the full B(GT) distribution.

  16. Sinusoidal Regge Oscillations from Short Lived Resonances

    NASA Astrophysics Data System (ADS)

    Sokolovski, D.; Felfli, Z.; Msezane, A. Z.

    2007-06-01

    It is well known that a resonance with a large angular life can produce sharp Breit-Wigner peaks in the energy dependence of integral cross sections [1,2]. Here we show that a short-lived resonance whose angular life is of order of one full rotation may produce a different kind of contribution to the integral cross section. This contribution has a sinousoidal form and its frequency is determined by the rotational constant of the complex. As one of the examples, we analyze the Regge oscillations observed in numerical simulations of the F+H2(v=0,j=0,φ=0) ->FH(v'=2,j'=0,φ'=0) + H reaction. In particular, we show that these oscillations are produced by two overlapping resonances located near the transition state and the van der Waals well, respectively [3]. [1] J. H. Macek, et al., Phys. Rev. Lett., 93, 183202, (2004). [2] Z. Felfli et al., J. Phys. B 39, L353 (2006) [3] D. Sokolovski, D. De Fazio, S. Cavalli and V. Aquilanti, J. Chem. Phys. (2007) (submitted).

  17. Delayed and In-beam Spectroscopy on Francium and Astatine Nuclei at the Proton Drip Line

    NASA Astrophysics Data System (ADS)

    Uusitalo, J.; Jakobsson, U.

    2011-11-01

    Delayed and in-beam spectroscopy on francium and astatine nuclei at and beyond the proton drip line has been performed. In neutron deficient astatine nuclei a shift to deformed shapes as a function of decreasing neutron has been obtained. In neutron deficient francium isotope the same shift is evident.

  18. Delayed and In-beam Spectroscopy on Francium and Astatine Nuclei at the Proton Drip Line

    SciTech Connect

    Uusitalo, J.; Jakobsson, U.; Collaboration: RITU-Gamma Gollaboration

    2011-11-30

    Delayed and in-beam spectroscopy on francium and astatine nuclei at and beyond the proton drip line has been performed. In neutron deficient astatine nuclei a shift to deformed shapes as a function of decreasing neutron has been obtained. In neutron deficient francium isotope the same shift is evident.

  19. Quadrupole Collectivity in Neutron Deficient Sn Isotopes

    NASA Astrophysics Data System (ADS)

    Gade, Alexandra

    2014-03-01

    One of the overarching goals of nuclear physics is the development of a comprehensive model of the atomic nucleus with predictive power across the nuclear chart. Of particular importance for the development of nuclear models is experimental data that consistently track the effect of isospin and changed binding, for example. The chain of Sn isotopes has been a formidable testing ground for nuclear models as some spectroscopic data is available from N = Z = 50 100Sn in the proximity of the proton dripline to 134Sn, beyond the very neutron-rich doubly magic nucleus 132Sn. In even-even nuclei, the electromagnetic quadrupole excitation strength is a measure of quadrupole collectivity, sensitive to the presence of shell gaps, nuclear deformation, and nucleon-nucleon correlations, for example. In the Sn isotopes, this transition strength has been reported from 104Sn to 130Sn, spanning a chain of 14 even-even Sn isotopes. The trend is asymmetric with respect to midshell and not even the largest-scale shell-model calculations have been able to describe the evolution of transition strength across the isotopic chain without varying effective charges. Implications will be discussed. This work was supported by the National Science Foundation under Grant No. PHY-1102511.

  20. Decay-Assisted Laser Spectroscopy of Neutron-Deficient Francium

    NASA Astrophysics Data System (ADS)

    Lynch, K. M.; Billowes, J.; Bissell, M. L.; Budinčević, I.; Cocolios, T. E.; De Groote, R. P.; De Schepper, S.; Fedosseev, V. N.; Flanagan, K. T.; Franchoo, S.; Garcia Ruiz, R. F.; Heylen, H.; Marsh, B. A.; Neyens, G.; Procter, T. J.; Rossel, R. E.; Rothe, S.; Strashnov, I.; Stroke, H. H.; Wendt, K. D. A.

    2014-01-01

    This paper reports on the hyperfine-structure and radioactive-decay studies of the neutron-deficient francium isotopes Fr202-206 performed with the Collinear Resonance Ionization Spectroscopy (CRIS) experiment at the ISOLDE facility, CERN. The high resolution innate to collinear laser spectroscopy is combined with the high efficiency of ion detection to provide a highly sensitive technique to probe the hyperfine structure of exotic isotopes. The technique of decay-assisted laser spectroscopy is presented, whereby the isomeric ion beam is deflected to a decay-spectroscopy station for alpha-decay tagging of the hyperfine components. Here, we present the first hyperfine-structure measurements of the neutron-deficient francium isotopes Fr202-206, in addition to the identification of the low-lying states of Fr202,204 performed at the CRIS experiment.

  1. Studies of images of short lived events using ERTS data

    NASA Technical Reports Server (NTRS)

    Deutschman, W. A. (Principal Investigator)

    1973-01-01

    The author has identified the following significant results. The program to study short-lived events with the ERTS-1 satellite has evaluated 97 events reported by the Center for Short-Lived Phenomena. Forty-eight of these events were listed as candidates for ERTS-1 coverage and 8 of these were considered significant enough to immediately alert the ERTS operation staff by telephone. Studies of the images received from six events indicate that useful data on short-lived events can be obtained from ERTS-1 that would be difficult or impossible to obtain by other methods.

  2. Collinear Resonance Ionization Spectroscopy of Neutron-Deficient Francium Isotopes

    NASA Astrophysics Data System (ADS)

    Flanagan, K. T.; Lynch, K. M.; Billowes, J.; Bissell, M. L.; Budinčević, I.; Cocolios, T. E.; de Groote, R. P.; De Schepper, S.; Fedosseev, V. N.; Franchoo, S.; Garcia Ruiz, R. F.; Heylen, H.; Marsh, B. A.; Neyens, G.; Procter, T. J.; Rossel, R. E.; Rothe, S.; Strashnov, I.; Stroke, H. H.; Wendt, K. D. A.

    2013-11-01

    The magnetic moments and isotope shifts of the neutron-deficient francium isotopes Fr202-205 were measured at ISOLDE-CERN with use of collinear resonance ionization spectroscopy. A production-to-detection efficiency of 1% was measured for Fr202. The background from nonresonant and collisional ionization was maintained below one ion in 105 beam particles. Through a comparison of the measured charge radii with predictions from the spherical droplet model, it is concluded that the ground-state wave function remains spherical down to Fr205, with a departure observed in Fr203 (N=116).

  3. Collinear resonance ionization spectroscopy of neutron-deficient francium isotopes.

    PubMed

    Flanagan, K T; Lynch, K M; Billowes, J; Bissell, M L; Budinčević, I; Cocolios, T E; de Groote, R P; De Schepper, S; Fedosseev, V N; Franchoo, S; Garcia Ruiz, R F; Heylen, H; Marsh, B A; Neyens, G; Procter, T J; Rossel, R E; Rothe, S; Strashnov, I; Stroke, H H; Wendt, K D A

    2013-11-22

    The magnetic moments and isotope shifts of the neutron-deficient francium isotopes (202-205)Fr were measured at ISOLDE-CERN with use of collinear resonance ionization spectroscopy. A production-to-detection efficiency of 1% was measured for (202)Fr. The background from nonresonant and collisional ionization was maintained below one ion in 10(5) beam particles. Through a comparison of the measured charge radii with predictions from the spherical droplet model, it is concluded that the ground-state wave function remains spherical down to (205)Fr, with a departure observed in (203)Fr (N=116). PMID:24313482

  4. Caffeine's Jolt Can Sometimes Be Short-Lived

    MedlinePlus

    ... page: https://medlineplus.gov/news/fullstory_159413.html Caffeine's Jolt Can Sometimes Be Short-Lived Stimulant effect ... 17, 2016 THURSDAY, June 16, 2016 (HealthDay News) -- Caffeine no longer improves alertness or mental performance after ...

  5. Unique and complementary information on shape coexistence in the neutron-deficient Pb region derived from Coulomb excitation

    NASA Astrophysics Data System (ADS)

    Wrzosek-Lipska, K.; Gaffney, L. P.

    2016-02-01

    Neutron-deficient isotopes of Pt-Hg-Pb-Po-Rn are the classic region in the investigation of shape coexistence in atomic nuclei. A large programme of Coulomb-excitation experiments has been undertaken at the REX-ISOLDE facility in CERN with a number of even-even isotopes in this region. These experiments have been used to probe the electromagnetic properties of yrast and non-yrast states of even-even exotic nuclei, above and below Z = 82. Amongst a large amount of different complementary techniques used to study nuclear structure, Coulomb excitation brings substantial and unique information detailing shape coexistence. In this paper we review the Coulomb-excitation campaign at REX-ISOLDE in the light-lead region together with most recently obtained results. Furthermore, we present some new interpretations that arise from this data and show testing comparisons to state-of-the-art nuclear models.

  6. New neutron-deficient isotopes from 78Kr fragmentation

    NASA Astrophysics Data System (ADS)

    Blank, B.; Goigoux, T.; Ascher, P.; Gerbaux, M.; Giovinazzo, J.; Grévy, S.; Kurtukian Nieto, T.; Magron, C.; Agramunt, J.; Algora, A.; Guadilla, V.; Montaner-Piza, A.; Morales, A. I.; Orrigo, S. E. A.; Rubio, B.; Ahn, D. S.; Doornenbal, P.; Fukuda, N.; Inabe, N.; Kiss, G.; Kubo, T.; Kubono, S.; Nishimura, S.; Phong, V. H.; Sakurai, H.; Shimizu, Y.; Söderström, P.-A.; Sumikama, T.; Suzuki, H.; Takeda, H.; Wu, J.; Fujita, Y.; Tanaka, M.; Gelletly, W.; Aguilera, P.; Molina, F.; Diel, F.; Lubos, D.; de Angelis, G.; Napoli, D.; Borcea, C.; Boso, A.; Cakirli, R. B.; Ganioglu, E.; Chiba, J.; Nishimura, D.; Oikawa, H.; Takei, Y.; Yagi, S.; Wimmer, K.; de France, G.; Go, S.

    2016-06-01

    In an experiment with the RIKEN projectile fragment separator called BigRIPS at the RIKEN Nishina Center, the fragmentation of a 78Kr beam allowed the observation of new neutron-deficient isotopes at the proton drip line. Clean identification spectra could be produced and 63Se,67Kr, and 68Kr were identified for the first time. In addition, 59Ge was also observed. Three of these isotopes, 59Ge,63Se, and 67Kr, are potential candidates for ground-state two-proton radioactivity. In addition, the isotopes 58Ge,62Se, and 66Kr were also sought but without success. The present experiment also allowed the determination of production cross sections for some of the most exotic isotopes. These measurements confirm the trend already observed that the empirical parametrization of fragmentation cross sections, EPAX, significantly overestimates experimental cross sections in this mass region.

  7. Beta-decay measurements of neutron-deficient cesium isotopes

    SciTech Connect

    Parry, R.F.

    1983-03-01

    Beta decay endpoint energy measurements of the neutron deficient cesium isotopes were done using an energy spectrum shape fitting technique. This was a departure from the typical method of endpoint energy analysis, the Fermi-Kurie plot. A discussion of the shape fitting procedure and its improved features are discussed. These beta endpoint measurements have led to total decay energies (Q/sub EC/) of the neutron deficient /sup 119/ /sup 123/Cs isotopes. The total decay energies of /sup 122m/Cs (Q/sub EC/ = 6.95 +- 0.25 MeV) and /sup 119/Cs (Q/sub EC/ = 6.26 +- 0.29 MeV) were new measurements. The total decay energies of /sup 123/Cs (Q/sub EC/ = 4.05 +- 0.18 MeV), /sup 122g/Cs (Q/sub EC/ = 7.05 +- 0.18 MeV), /sup 121/Cs (Q/sub EC/ = 5.21 +- 0.22 MeV), and /sup 120/Cs (Q/sub EC/ = 7.38 +- 0.23 MeV) were measurements with significantly improved uncertainties as compared to the literature. Further, a combination of the energy levels derived from previous literature gamma-gamma coincident measurements and the experimental beta-coincident gamma decay energies has supported an improved level scheme for /sup 121/Xe and the proposal of three new energy levels in /sup 119/Xe. Comparison of the experimental cesium mass excesses (determined with our Q/sub EC/ values and known xenon mass excesses) with both the literature and theoretical predicted values showed general agreement except for /sup 120/Cs. Possible explanations for this deviation are discussed.

  8. Soot and short-lived pollutants provide political opportunity

    NASA Astrophysics Data System (ADS)

    Victor, David G.; Zaelke, Durwood; Ramanathan, Veerabhadran

    2015-09-01

    Cutting levels of soot and other short-lived pollutants delivers tangible benefits and helps governments to build confidence that collective action on climate change is feasible. After the Paris climate meeting this December, actually reducing these pollutants will be essential to the credibility of the diplomatic process.

  9. Nuclear fission of neutron-deficient protactinium nuclides

    SciTech Connect

    Nishinaka, I.; Nagame, Y.; Tsukada, K.; Ikezoe, H.; Sueki, K.; Nakahara, H.; Tanikawa, M.; Ohtsuki, T.

    1997-08-01

    Fragment velocity, kinetic energy, mass yield, and element yield distributions in the fission of neutron-deficient Pa isotopes produced in the reactions of {sup 16}O and {sup 18}O on {sup 209}Bi have been measured at incident beam energies near and above the Coulomb barriers by the time-of-flight and radiochemical methods. An asymmetric mass-division component has been observed. Measured fission cross sections were compared with the results of statistical model calculations which take into account two fission barrier heights for symmetric and asymmetric yields. The fission barrier height deduced for the asymmetric fission is found slightly lower than that for the symmetric one. The difference between the two barrier heights in the fission of the present protactinium nuclides (N{approximately}135) is considerably smaller than that in the neutron-rich nuclide of {sup 233}Pa (N{approximately}142), indicating that the difference sensitively depends on the neutron number of the fissioning nuclide. {copyright} {ital 1997} {ital The American Physical Society}

  10. Investigation of the structure of neutron-deficient Cd isotopes

    NASA Astrophysics Data System (ADS)

    Simon, Anna; Humby, P.; Beausang, C. W.; Burke, J. T.; Casperson, R. J.; McCleskey, M.; Saastamoinen, A.; Allmond, J. M.; Chyzh, R.; Dag, M.; Koglin, J.; Ota, S.; Ross, T. J.

    2014-03-01

    The STARLITER setup at Texas A&M University consists of an array of six Compton suppressed HPGe clover γ-ray detectors coupled with a segmented Si ΔE-E charged particle telescope. The combination allows for coincident γ ray and particle spectroscopy and provides a powerful tool for precise determination of the nuclear level structure. A recent experiment conducted using STARLITER aimed at the investigation of structures of neutron-deficient Cd isotopes (A = 104, 105, 106) using an enriched 106Cd target and 35 MeV proton beam supplied by the K-150 Cyclotron at TAMU. Low mass cadmium isotopes are a great environment for analysis of the evolution from vibrational to rotational sequences in A ~100-110 region and provide insight into the structure phenomena around Z = 50 shell closure. Here, the first results of the experiment will be presented. This work was partly supported by the US Department of Energy Grants No. DE-FG52-06NA26206 and No. DE-FG02-05ER41379.

  11. Short-lived positron emitter labeled radiotracers - present status

    SciTech Connect

    Fowler, J.S.; Wolf, A.P.

    1982-01-01

    The preparation of labelled compounds is important for the application of positron emission transaxial tomography (PETT) in biomedical sciences. This paper describes problems and progress in the synthesis of short-lived positron emitter (/sup 11/C, /sup 18/F, /sup 13/N) labelled tracers for PETT. Synthesis of labelled sugars, amino acids, and neurotransmitter receptors (pimozide and spiroperidol tagged with /sup 11/C) is discussed in particular. (DLC)

  12. New Short-Lived Isotope 221U and the Mass Surface Near N =126

    NASA Astrophysics Data System (ADS)

    Khuyagbaatar, J.; Yakushev, A.; Düllmann, Ch. E.; Ackermann, D.; Andersson, L.-L.; Block, M.; Brand, H.; Cox, D. M.; Even, J.; Forsberg, U.; Golubev, P.; Hartmann, W.; Herzberg, R.-D.; Heßberger, F. P.; Hoffmann, J.; Hübner, A.; Jäger, E.; Jeppsson, J.; Kindler, B.; Kratz, J. V.; Krier, J.; Kurz, N.; Lommel, B.; Maiti, M.; Minami, S.; Mistry, A. K.; Mrosek, Ch. M.; Pysmenetska, I.; Rudolph, D.; Sarmiento, L. G.; Schaffner, H.; Schädel, M.; Schausten, B.; Steiner, J.; De Heidenreich, T. Torres; Uusitalo, J.; Wegrzecki, M.; Wiehl, N.; Yakusheva, V.

    2015-12-01

    Two short-lived isotopes 221U and 222U were produced as evaporation residues in the fusion reaction 50Ti + 176Yb at the gas-filled recoil separator TASCA. An α decay with an energy of Eα=9.31 (5 ) MeV and half-life T1 /2=4.7 (7 ) μ s was attributed to 222U. The new isotope 221U was identified in α -decay chains starting with Eα=9.71 (5 ) MeV and T1 /2=0.66 (14 ) μ s leading to known daughters. Synthesis and detection of these unstable heavy nuclei and their descendants were achieved thanks to a fast data readout system. The evolution of the N =126 shell closure and its influence on the stability of uranium isotopes are discussed within the framework of α -decay reduced width.

  13. Measures Urged to Cut Short-Lived Climate Pollutants

    NASA Astrophysics Data System (ADS)

    Showstack, Randy

    2013-03-01

    To produce significant near-term climate benefits, the Obama administration should take a series of actions under existing authorities to reduce greenhouse gases that have relatively short atmospheric lifetimes of weeks to a few decades, according to a 12 March study by the nonprofit Center for Climate and Energy Solutions (C2ES). The report, "Domestic Policies to Reduce the Near-Term Risks of Climate Change," notes that recent estimates suggest that about 30-40% of warming experienced to date can be attributed to these short-lived pollutants, which include black carbon, methane, and hydrofluorocarbons (HFCs).

  14. SHORT-LIVED RADIO BURSTS FROM THE CRAB PULSAR

    SciTech Connect

    Crossley, J. H.; Eilek, J. A.; Hankins, T. H.; Kern, J. S.

    2010-10-20

    Our high-time-resolution observations reveal that individual main pulses from the Crab pulsar contain one or more short-lived microbursts. Both the energy and duration of bursts measured above 1 GHz can vary dramatically in less than a millisecond. These fluctuations are too rapid to be caused by propagation through turbulence in the Crab Nebula or in the interstellar medium; they must be intrinsic to the radio emission process in the pulsar. The mean duration of a burst varies with frequency as {nu}{sup -2}, significantly different from the broadening caused by interstellar scattering. We compare the properties of the bursts to some simple models of microstructure in the radio emission region.

  15. Near-Term Climate Mitigation by Short-Lived Forcers

    SciTech Connect

    Smith, Steven J.; Mizrahi, Andrew H.

    2013-08-12

    Emissions reductions focused on anthropogenic climate forcing agents with relatively short atmospheric lifetimes such as methane (CH4) and black carbon (BC) have been suggested as a strategy to reduce the rate of climate change over the next several decades. We find that reductions of methane and BC would likely have only a modest impact on near-term climate warming. Even with maximally feasible reductions phased in from 2015 to 2035, global mean temperatures in 2050 are reduced by 0.16 °C, with an uncertainty range of 0.04-0.36°C, with the high end of this range only possible if total historical aerosol forcing is small. More realistic mitigation scenarios would likely provide a smaller climate benefit. The climate benefits from targeted reductions in short-lived forcing agents are smaller than previously estimated and are not substantially different in magnitude from the benefits due to a comprehensive climate policy.

  16. Nucleosynthesis of Short-lived Radioactivities in Massive Stars

    NASA Technical Reports Server (NTRS)

    Meyer, B. S.

    2004-01-01

    A leading model for the source of many of the short-lived radioactivities in the early solar nebula is direct incorporation from a massive star [1]. A recent and promising incarnation of this model includes an injection mass cut, which is a boundary between the stellar ejecta that become incorporated into the solar cloud and those ejecta that do not [2-4]. This model also includes a delay time between ejection from the star and incorporation into early solar system solid bodies. While largely successful, this model requires further validation and comparison against data. Such evaluation becomes easier if we have a better sense of the nature of the synthesis of the various radioactivities in the star. That is the goal of this brief abstract.

  17. Study of asymmetric fission yield behavior from neutron-deficient Hg isotope

    SciTech Connect

    Perkasa, Y. S.; Waris, A. Kurniadi, R. Su'ud, Z.

    2014-09-30

    A study of asymmetric fission yield behavior from a neutron-deficient Hg isotope has been conducted. The fission yield calculation of the neutron-deficient Hg isotope using Brownian Metropolis shape had showed unusual result at decreasing energy. In this paper, this interesting feature will be validated by using nine degree of scission shapes parameterization from Brosa model that had been implemented in TALYS nuclear reaction code. This validation is intended to show agreement between both model and the experiment result. The expected result from these models considered to be different due to dynamical properties that implemented in both models.

  18. Quantifying Short-Lived Events in Multistate Ionic Current Measurements

    PubMed Central

    2015-01-01

    We developed a generalized technique to characterize polymer–nanopore interactions via single channel ionic current measurements. Physical interactions between analytes, such as DNA, proteins, or synthetic polymers, and a nanopore cause multiple discrete states in the current. We modeled the transitions of the current to individual states with an equivalent electrical circuit, which allowed us to describe the system response. This enabled the estimation of short-lived states that are presently not characterized by existing analysis techniques. Our approach considerably improves the range and resolution of single-molecule characterization with nanopores. For example, we characterized the residence times of synthetic polymers that are three times shorter than those estimated with existing algorithms. Because the molecule’s residence time follows an exponential distribution, we recover nearly 20-fold more events per unit time that can be used for analysis. Furthermore, the measurement range was extended from 11 monomers to as few as 8. Finally, we applied this technique to recover a known sequence of single-stranded DNA from previously published ion channel recordings, identifying discrete current states with subpicoampere resolution. PMID:24397836

  19. Studies of Neutron-Deficient Nuclei Near the Z = 82 Shell Closure via Cold Fusion Reactions

    NASA Astrophysics Data System (ADS)

    Carpenter, M. P.; Kondev, F. G.; Janssens, R. V. F.; Seweryniak, D.; Khoo, T. L.; Lauritsen, T.; Lister, C. J.; Zhu, S.; Camera, F.; Bracco, A.; Million, B.; Leoni, S.; Jenkins, D. G.; Wadsworth, R.

    2009-03-01

    Over the last decade, we have performed in-beam experiments using Gammasphere+FMA to measure excited states in proton-rich Au, Hg, Tl and Pb isotopes. In these studies, the use of the FMA is essential in order to differentiate evaporation residues from the large fission background which dominates the reaction cross-section. In addition, we have found that using near-symmetric reactions at bombarding energies near the Coloumb barrier is beneficial in performing these studies. By keeping the bombarding energy low, fission is minimized and the reaction products are concentrated in only a few channels. New results have recently been obtained using the 90Zr+92Mo reaction to study shape co-existence in 181Tl via the lp evaporation channel. In addition, we have measured the total γ-ray energy and multiplicity associated with the surviving compund system, 179Au, following the fusion reaction, 90Zr+89Y.

  20. Particle decay of very neutron deficient nuclei near {sup 100}Sn

    SciTech Connect

    Tighe, R.J.; Moltz, D.M.; Batchelder, J.C.; Ognibene, T.J.; Rowe, M.W.; Cerny, J.

    1993-10-01

    Proton emission from the nuclear ground state (gs) not only determines the limit of nuclear stability, but yields information on nuclear masses and structure very far from stability. There has been much recent experimental work in the region of the expected doubly-magic nucleus {sup 100}Sn (N=Z=50). This includes the discovery of the lightest known gs proton emitters, {sup 109}I and {sup 113}CS. We have used the compound nuclear reaction {sup 58}Ni + {sup 50}Cr to search for the gs particle decay of {sup 104}Sb and {sup 105}Sb. The evaporation residues were transported via our He-jet system and collected on a thin tape at the center of our new detector ball. This detector ball consists of six gas-{Delta}E gas-{Delta}E Si-E triple telescopes each capable of detecting protons with energies down to {approx}200 keV. Previous attempts to identify the gs proton decay of {sup 105}Sb had a lower energy threshold of {approx}500 keV. We have observed several low-energy ({approx}350-800 keV) proton groups at {sup 58}Ni bombarding energies of 223 MeV, 244 MeV, and 259 MeV.

  1. Short-lived proton radioactivity studies at HRIBF

    SciTech Connect

    Batchelder, J. C.; Bingham, C. R.; Ginter, T. N.; Gross, C. J.; Grzywacz, R.; Karny, M.; Janas, Z.; Mas, F.; McConnell, J. W.; Rykaczewski, K.; Toth, K. S.; Piechaczek, A.; Zganjar, E. F.; Semmes, P.

    1999-11-16

    An accurate determination of the experimental spectroscopic factor of proton emitting nuclei precisely defines the main component of the proton wave function for the unbound state. However, this has proven difficult for nuclei with Z{<=}71 due to the unknown beta-branching ratios involved. One way to solve this problem is to study proton-emitters with half-lives far too short for beta-emission to compete. Recent work at the Holifield Radioactive Ion Beam Facility has produced information on {sup 141m}Ho, {sup 145}Tm, {sup 150m}Lu and {sup 151m}Lu, all of which have half-lives in the {mu}s region. A comparison between calculated and experimental spectroscopic factors for these nuclei is given.

  2. Decay studies of the highly neutron-deficient indium isotopes

    SciTech Connect

    Wouters, J.M.

    1982-02-01

    An extension of the experimentally known nuclidic mass surface to nuclei far from the region of beta-stability is of fundamental interest in providing a better determination of the input parameters for the various nuclear mass formulae, allowing a more accurate prediction of the ultimate limits of nuclear stability. In addition, a study of the shape of the mass surface in the vicinity of the doubly-closed nuclide /sup 100/Sn provides initial information on the behavior of the shell closure to be expected when Z = N = 50. Experiments measuring the decay energies of /sup 103/ /sup 105/In by ..beta..-endpoint measurements are described with special attention focused on the development of a plastic scintillator ..beta..-telescope coupled to the on-line mass separator RAMA (Recoil Atom Mass Analyzer). An attempt to measure the ..beta..-endpoint energy of /sup 102/In is also briefly described. The experimentally determined decay energies and derived masses for /sup 103/ /sup 105/In are compared with the predictions of different mass models to identify which models are more successful in this region. Furthermore, the inclusion in these comparisons of the available data on the neutron-rich indium nuclei permits a systematic study of their ground state mass behavior as a function of the neutron number between the shell closures at N = 50 and N = 82. These analyses indicate that the binding energy of /sup 103/In is 1 MeV larger than predicted by the majority of the mass models. An examination of the Q/sub EC/ surface and the single- and two-neutron separation energies in the vicinity of /sup 103/ /sup 105/In is also performed to investigate further the deviation and other possible systematic variations in the mass surface in a model-independent way.

  3. Convective transport of very short lived bromocarbons to the stratosphere

    NASA Astrophysics Data System (ADS)

    Liang, Q.; Atlas, E.; Blake, D.; Dorf, M.; Pfeilsticker, K.; Schauffler, S.

    2014-06-01

    We use the NASA Goddard Earth Observing System (GEOS) Chemistry Climate Model (GEOSCCM) to quantify the contribution of the two most important brominated very short lived substances (VSLSs), bromoform (CHBr3) and dibromomethane (CH2Br2), to stratospheric bromine and its sensitivity to convection strength. Model simulations suggest that the most active transport of VSLSs from the marine boundary layer through the tropopause occurs over the tropical Indian Ocean, the tropical western Pacific, and off the Pacific coast of Mexico. Together, convective lofting of CHBr3 and CH2Br2 and their degradation products supplies ~8 ppt total bromine to the base of the tropical tropopause layer (TTL, ~150 hPa), similar to the amount of VSLS organic bromine available in the marine boundary layer (~7.8-8.4 ppt) in the active convective lofting regions mentioned above. Of the total ~8 ppt VSLS bromine that enters the base of the TTL at ~150 hPa, half is in the form of organic source gases and half in the form of inorganic product gases. Only a small portion (<10%) of the VSLS-originated bromine is removed via wet scavenging in the TTL before reaching the lower stratosphere. On average, globally, CHBr3 and CH2Br2 together contribute ~7.7 pptv to the present-day inorganic bromine in the stratosphere. However, varying model deep-convection strength between maximum (strongest) and minimum (weakest) convection conditions can introduce a ~2.6 pptv uncertainty in the contribution of VSLSs to inorganic bromine in the stratosphere (BryVSLS). Contrary to conventional wisdom, the minimum convection condition leads to a larger BryVSLS as the reduced scavenging in soluble product gases, and thus a significant increase in product gas injection (2-3 ppt), greatly exceeds the relatively minor decrease in source gas injection (a few 10ths ppt).

  4. Deformation in the neutron-deficient rare earth isotopes: Radioactive decay scheme studies in the neodymium, promethium, and samarium isotopes

    SciTech Connect

    Breitenbach, J.B.

    1993-12-31

    Several experiments were performed at the UNISOR isotope separator facility at HHIRF at the Oak Ridge National Laboratory on the {beta}{sup +}/EC decay of neutron-deficient rare earth isotopes. Data for the decay chain {sup 133}Sm {yields} {sup 133}Pm {yields} {sup 133}Nd was obtained, consisting of multiscaled spectra of {gamma} rays, X rays, and conversion electrons, as well as {gamma}{gamma}t, X{gamma}t, e{gamma}t and eXt coincidences. Gamma rays associated with the decay of {sup 133}Sm and {sup 133}Pm were observed for the first time. The decay of a new low-spin (1/2) isomeric state, with a half life of about 70 sec was established for {sup 133}Nd. The level schemes for {sup 133}Nd and {sup 133}Pr were constructed. An M3 and two E1 isomers are established in {sup 133}Nd and an E3 isomer is confirmed in {sup 133}Pr. The energy level systematics for the nuclear region bounded by Z {ge} 58 and N {le} 78 is discussed. Theoretical interpretations are based on the particle-plus-triaxial rotor model calculations. In the framework of these calculations, the {beta}{sub 2} deformation is moderate for these nuclei ({beta}{sub 2} {approx} 0.20-0.25). A sudden onset of strong deformation is not observed, in contrast with the theoretical predictions by Leander and Moeller [Lea82].

  5. New Short-Lived Isotope ^{221}U and the Mass Surface Near N=126.

    PubMed

    Khuyagbaatar, J; Yakushev, A; Düllmann, Ch E; Ackermann, D; Andersson, L-L; Block, M; Brand, H; Cox, D M; Even, J; Forsberg, U; Golubev, P; Hartmann, W; Herzberg, R-D; Heßberger, F P; Hoffmann, J; Hübner, A; Jäger, E; Jeppsson, J; Kindler, B; Kratz, J V; Krier, J; Kurz, N; Lommel, B; Maiti, M; Minami, S; Mistry, A K; Mrosek, Ch M; Pysmenetska, I; Rudolph, D; Sarmiento, L G; Schaffner, H; Schädel, M; Schausten, B; Steiner, J; De Heidenreich, T Torres; Uusitalo, J; Wegrzecki, M; Wiehl, N; Yakusheva, V

    2015-12-11

    Two short-lived isotopes ^{221}U and ^{222}U were produced as evaporation residues in the fusion reaction ^{50}Ti+^{176}Yb at the gas-filled recoil separator TASCA. An α decay with an energy of E_{α}=9.31(5)  MeV and half-life T_{1/2}=4.7(7)  μs was attributed to ^{222}U. The new isotope ^{221}U was identified in α-decay chains starting with E_{α}=9.71(5)  MeV and T_{1/2}=0.66(14)  μs leading to known daughters. Synthesis and detection of these unstable heavy nuclei and their descendants were achieved thanks to a fast data readout system. The evolution of the N=126 shell closure and its influence on the stability of uranium isotopes are discussed within the framework of α-decay reduced width. PMID:26705628

  6. Crantor, a short-lived horseshoe companion to Uranus

    NASA Astrophysics Data System (ADS)

    de la Fuente Marcos, C.; de la Fuente Marcos, R.

    2013-03-01

    Context. Stable co-orbital motion with Uranus is vulnerable to planetary migration, but temporary co-orbitals may exist today. So far, only two candidates have been suggested, both moving on horseshoe orbits: 83982 Crantor (2002 GO9) and 2000 SN331. Aims: (83982) Crantor is currently classified in the group of the Centaurs by the MPC although the value of its orbital period is close to that of Uranus. Here we revisit the topic of the possible 1:1 commensurability of (83982) Crantor with Uranus, explore its dynamical past, and look into its medium-term stability and future orbital evolution. Methods: Our analysis is based on the results of N-body calculations that use the most updated ephemerides and include perturbations by the eight major planets, the Moon, the barycenter of the Pluto-Charon system, and the three largest asteroids. Results: (83982) Crantor currently moves inside Uranus' co-orbital region on a complex horseshoe orbit. The motion of this object is primarily driven by the influence of the Sun and Uranus, although Saturn plays a significant role in destabilizing its orbit. The precession of the nodes of (83982) Crantor, which is accelerated by Saturn, controls its evolution and short-term stability. Although this object follows a temporary horseshoe orbit, more stable trajectories are possible and we present 2010 EU65 as a long-term horseshoe librator candidate in urgent need of follow-up observations. Available data indicate that the candidate 2000 SN331 is not a Uranus' co-orbital. Conclusions: Our calculations confirm that (83982) Crantor is currently trapped in the 1:1 commensurability with Uranus but it is unlikely to be a primordial 1:1 librator. Although this object follows a chaotic, short-lived horseshoe orbit, longer term horseshoe stability appears to be possible. We also confirm that high-order resonances with Saturn play a major role in destabilizing the orbits of Uranus co-orbitals. Figures 2 and 6 (animations) are available in

  7. Efficiency of short-lived halogens at influencing climate through depletion of stratospheric ozone

    NASA Astrophysics Data System (ADS)

    Hossaini, R.; Chipperfield, M. P.; Montzka, S. A.; Rap, A.; Dhomse, S.; Feng, W.

    2015-03-01

    Halogens released from long-lived anthropogenic substances, such as chlorofluorocarbons, are the principal cause of recent depletion of stratospheric ozone, a greenhouse gas. Recent observations show that very short-lived substances, with lifetimes generally under six months, are also an important source of stratospheric halogens. Short-lived bromine substances are produced naturally by seaweed and phytoplankton, whereas short-lived chlorine substances are primarily anthropogenic. Here we used a chemical transport model to quantify the depletion of ozone in the lower stratosphere from short-lived halogen substances, and a radiative transfer model to quantify the radiative effects of that ozone depletion. According to our simulations, ozone loss from short-lived substances had a radiative effect nearly half that from long-lived halocarbons in 2011 and, since pre-industrial times, has contributed a total of about -0.02 W m-2 to global radiative forcing. We find natural short-lived bromine substances exert a 3.6 times larger ozone radiative effect than long-lived halocarbons, normalized by halogen content, and show atmospheric levels of dichloromethane, a short-lived chlorine substance not controlled by the Montreal Protocol, are rapidly increasing. We conclude that potential further significant increases in the atmospheric abundance of short-lived halogen substances, through changing natural processes or continued anthropogenic emissions, could be important for future climate.

  8. Studies of images of short-lived events using ERTS data

    NASA Technical Reports Server (NTRS)

    Deutschman, W. A. (Principal Investigator)

    1973-01-01

    The author has identified the following significant results. Significant results are the continued detection of short-lived events. The following have been detected and analyzed: forest fires, oil spills, vegetation damage, volcanoes, storm ridges, and earthquakes. It is hoped that the Mississippi River flood scenes will arrive shortly and then floods be added to the list of identified short-lived events.

  9. Studies of images of short-lived events using ERTS data

    NASA Technical Reports Server (NTRS)

    Deutschman, W. A. (Principal Investigator)

    1973-01-01

    The author has identified the following significant results. Of significance are the continued detection and analysis of such short-lived events as forest fires, oil spills, vegetation damage, volcanoes, storm ridges, and earthquakes.

  10. Existence of long-lived isomeric states in naturally-occurring neutron-deficient Th isotopes

    SciTech Connect

    Marinov, A.; Kashiv, Y.; Rodushkin, I.; Halicz, L.; Segal, I.; Pape, A.; Miller, H. W.; Kolb, D.; Brandt, R.

    2007-08-15

    Four long-lived neutron-deficient Th isotopes with atomic mass numbers 211 to 218 and abundances of (1-10)x10{sup -11} relative to {sup 232}Th have been found in a study of naturally-occurring Th using inductively coupled plasma-sector field mass spectrometry. It is deduced that long-lived isomeric states exist in these isotopes. The hypothesis that they might belong to a new class of long-lived high spin super- and hyperdeformed isomeric states is discussed.

  11. Nuclear moments and charge radii of neutron-deficient francium isotopes and isomers

    NASA Astrophysics Data System (ADS)

    Voss, A.; Buchinger, F.; Cheal, B.; Crawford, J. E.; Dilling, J.; Kortelainen, M.; Kwiatkowski, A. A.; Leary, A.; Levy, C. D. P.; Mooshammer, F.; Ojeda, M. L.; Pearson, M. R.; Procter, T. J.; Tamimi, W. Al

    2015-04-01

    Collinear laser fluorescence spectroscopy has been performed on the ground and isomeric states of Fr,206204 in order to determine their spins, nuclear moments, and changes in mean-squared charge radii. A new experimental technique has been developed as part of this work which much enhances the data collection rate while maintaining the high resolution. This has permitted the extension of this study to the two isomeric states in each nucleus. The investigation of nuclear g factors and mean-squared charge radii indicates that the neutron-deficient Fr isotopes lie in a transitional region from spherical towards more collective structures.

  12. {alpha} decay studies of very neutron-deficient francium and radium isotopes

    SciTech Connect

    Uusitalo, J.; Leino, M.; Enqvist, T.; Grahn, T.; Greenlees, P.T.; Jones, P.; Julin, R.; Juutinen, S.; Keenan, A.; Kettunen, H.; Koivisto, H.; Kuusiniemi, P.; Leppaenen, A.-P.; Nieminen, P.; Pakarinen, J.; Rahkila, P.; Scholey, C.; Eskola, K.

    2005-02-01

    Very neutron-deficient francium and radium isotopes have been produced in fusion evaporation reactions using {sup 63}Cu and {sup 65}Cu ions on {sup 141}Pr targets and {sup 36}Ar ions on {sup 170}Yb targets. The gas-filled recoil separator RITU was employed to collect the fusion products and to separate them from the scattered beam. The activities were implanted into a position-sensitive silicon detector after passing through a gas-counter system. The isotopes were identified using spatial and time correlations between the implants and decays. Two new {alpha} decaying radium isotopes, {sup 201}Ra and {sup 202}Ra, were identified. The {alpha} decay energy and half-life of {sup 203}Ra were measured with improved precision. The {alpha} decay properties measured for the francium isotopes {sup 201}Fr,{sup 202}Fr,{sup 203}Fr, and {sup 204}Fr were confirmed, in many cases with improved precision. For the first time, a ({pi}s{sub 1/2}{sup -1})1/2{sup +} proton intruder state was identified in francium isotopes, namely in {sup 201}Fr and tentatively in {sup 203}Fr. The measured decay properties for the neutron-deficient odd-mass Fr isotopes suggest an onset of substantial deformation at N=112.

  13. α decay of the very neutron-deficient isotopes 197-199Fr

    NASA Astrophysics Data System (ADS)

    Kalaninová, Z.; Andreyev, A. N.; Antalic, S.; Heßberger, F. P.; Ackermann, D.; Andel, B.; Drummond, M. C.; Hofmann, S.; Huyse, M.; Kindler, B.; Lane, J. F. W.; Liberati, V.; Lommel, B.; Page, R. D.; Rapisarda, E.; Sandhu, K.; Šáro, Š.; Thornthwaite, A.; Van Duppen, P.

    2013-04-01

    Decay properties of the very neutron-deficient isotopes 197-199Fr were studied at the velocity filter Separator for Heavy Ion reaction Products (SHIP) at GSI in Darmstadt. The isotopes were produced in the 2n-4n evaporation channels of the fusion-evaporation reaction 60Ni+141Pr → 201Fr*. Improved α-decay properties of 199Fr were determined and the possible existence of two α-decaying states in this nucleus is discussed. For the isotope 198Fr a broad α-decay energy distribution was detected in the range of (7470-7930) keV and two α-decaying states were observed with half-lives of 1.1(7) and 15(3) ms. The new isotope 197Fr was identified based on the observation of one α-decay chain yielding Eα=7728(15) keV and T1/2=0.6-0.3+3.0 ms. The systematics of reduced α-decay widths are presented for neutron-deficient francium, radon, and astatine isotopes.

  14. Possibilities of production of neutron-deficient isotopes of U, Np, Pu, Am, Cm, and Cf in complete fusion reactions

    SciTech Connect

    Adamian, G. G.; Antonenko, N. V.; Zubov, A. S.; Scheid, W.

    2008-10-15

    Within the dinuclear system model we analyze the production of yet unknown neutron-deficient isotopes of U, Np, Pu, Am, Cm, and Cf in various complete fusion reactions. Different deexcitation channels of the excited compound nucleus are treated. The results are obtained without special adjustment to the selected evaporation channel. The fusion probability is an important ingredient of the excitation function. The results are in good agreement with the available experimental data. The alpha decay half-life times in the neutron-deficient actinides are discussed.

  15. Nuclear Reactions on Unstable Nuclei and the Surrogate Reaction Technique

    SciTech Connect

    Escher, J

    2004-03-01

    Determining reaction cross sections on short-lived nuclear species is a major challenge for nuclear physics and nuclear astrophysics. Many of these nuclei are too difficult to produce with currently available experimental techniques or too short-lived to serve as targets in present-day set-ups. Some nuclear reactions will remain immeasurable even at upcoming and planned radioactive beam facilities. It is therefore important to explore alternative methods for determining reaction cross sections on unstable nuclei.

  16. Superdeformation in the mercury nuclei

    SciTech Connect

    Janssens, R.V.F.; Carpenter, M.P.; Fernandez, P.B.; Moore, E.F.; Ahmad, I.; Khoo, T.L.; Wolfs, F.L.H. ); Drigert, M.W. ); Ye, D.; Beard, K.B.; Garg, U.; Reviol, W. ); Bearden, I.G.; Benet, P.; Daly, P.J.; Grabowski, Z.W. )

    1990-01-01

    We shall first summarize the present experimental situation concerning {sup 192}Hg, the nucleus regarded as the analog of {sup 152}Dy for this superdeformation (SD) region in that gaps are calculated to occur at large deformation for Z = 80 and N = 112. Proton and neutron excitations out of the {sup 192}Hg core will then be reviewed with particular emphasis on {sup 191}Hg and {sup 193}Tl. The presentation will conclude with a brief discussion on limits of the SD region for neutron deficient Hg nuclei. 26 refs., 10 figs.

  17. Mass measurements of short-lived isotopes in a penning trap

    SciTech Connect

    Kern, F.; Egelhof, P.; Hilberath, T.; Kalinowsky, H.; Kluge, H.h.; Kunz, K.; Schweikhard, L.; Stolzenberg, H.; Moore, R.B.; Audi, G.; and others

    1987-12-10

    A mass spectrometer has been set up at the on-line isotope separator ISOLDE at CERN/Geneva. Mass-separated radioactive ions are stored in a Penning trap. Their mass is determined by a measurement of the cyclotron frequency in the magnetic field of a superconducting magnet. A resolving power of up to 300.000 and a precision of some 10 keV were determined in case of mass measurements of neutron-deficient RB and Cs isotopes. The resonance of the isobars /sup 88/Sr and /sup 88/Rb were clearly resolved and evidence was obtained for an isomer in /sup 122/Cs.

  18. A technique for the measurement of electron attachment to short-lived excited species

    SciTech Connect

    Christophorou, L.G.; Pinnaduwage, L.A. ); Bitouni, A.P. . Dept. of Physics)

    1990-01-01

    A technique is described for the measurement of electron attachment to short-lived ({approx lt}10{sup {minus}9} s) excited species. Preliminary results are presented for photoenhanced electron attachment to short-lived electronically-excited states of triethylamine molecules produced by laser two-photon excitation. The attachment cross sections for these excited states are estimated to be >10{sup {minus}11} cm{sup 2} and are {approximately}10{sup 7} larger compared to those for the unexcited (ground-state) molecules. 8 refs., 4 figs.

  19. Rotation induced octupole correlations in the neutron-deficient 109Te nucleus

    NASA Astrophysics Data System (ADS)

    de Angelis, G.; Fahlander, C.; Gadea, A.; Farnea, E.; Bazzacco, D.; Belcari, N.; Blasi, N.; Bizzeti, P. G.; Bizzeti-Sona, A.; de Acuña, D.; de Poli, M.; Grawe, H.; Johnson, A.; Lo Bianco, G.; Lunardi, S.; Napoli, D. R.; Nyberg, J.; Pavan, P.; Persson, J.; Rossi Alvarez, C.; Rudolph, D.; Schubart, R.; Spolaore, P.; Wyss, R.; Xu, F.

    1998-10-01

    High spin states in the neutron deficient nucleus 109Te have been populated with the 58Ni+54Fe reaction at 220 MeV and investigated through γ-spectroscopy methods at the GASP spectrometer making use of reaction channel selection with the ISIS Si-ball. The level scheme has been extended up to an excitation energy of ~12.1 MeV. The spins and parities of the observed levels are assigned tentatively supporting the identification of two bands of opposite parity connected by strong dipole transitions inferred to be of E1 character. Octupole correlations in 109Te induced by rotation are suggested as the cause of this effect.

  20. First direct mass measurement of the neutron-deficient nucleus 24Al

    NASA Astrophysics Data System (ADS)

    Chowdhury, U.; Leach, K. G.; Andreoiu, C.; Bader, A.; Brodeur, M.; Chaudhuri, A.; Gallant, A. T.; Grossheim, A.; Gwinner, G.; Klawitter, R.; Kwiatkowski, A. A.; Lennarz, A.; Macdonald, T. D.; Pearkes, J.; Schultz, B. E.; Dilling, J.

    2015-10-01

    The first direct mass measurement of the neutron-deficient nucleus 24Al was performed via Penning-Trap Mass Spectrometry (PTMS) using TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This measurement was facilitated by the use of TRIUMF's new Ion-Guide Laser Ion Source (IG-LIS), which reduced A =24 isobaric contamination in the delivered beam by nearly six orders of magnitude. The measured mass excess was found to be Δ =-48.86 (23 ) keV, which is five times more precise than the value quoted in the most recent atomic mass evaluation. When combined with the relevant 24Al excitation energy, and a recent measurement of the 23Mg mass, the astrophysical 23Mg(p,γ ) 24Al reaction resonance energy is extracted as Er=480.8 (14 ) keV. The presented value shows a 2 σ disagreement with the direct measurement of this quantity by the DRAGON recoil spectrometer.

  1. High-precision masses of neutron-deficient rubidium isotopes using a Penning trap mass spectrometer

    SciTech Connect

    Kellerbauer, A.; Audi, G.; Guenaut, C.; Lunney, D.; Beck, D.; Herfurth, F.; Kluge, H.-J.; Weber, C.; Yazidjian, C.; Blaum, K.; Bollen, G.; Schwarz, S.; Herlert, A.; Schweikhard, L.

    2007-10-15

    The atomic masses of the neutron-deficient radioactive rubidium isotopes {sup 74-77,79,80,83}Rb have been measured with the Penning trap mass spectrometer ISOLTRAP. Using the time-of-flight cyclotron resonance technique, relative mass uncertainties ranging from 1.6x10{sup -8} to 5.6x10{sup -8} were achieved. In all cases, the mass precision was significantly improved as compared with the prior Atomic-Mass Evaluation; no significant deviations from the literature values were observed. The exotic nuclide {sup 74}Rb, with a half-life of only 65 ms, is the shortest-lived nuclide on which a high-precision mass measurement in a Penning trap has been carried out. The significance of these measurements for a check of the conserved-vector-current hypothesis of the weak interaction and the unitarity of the Cabibbo-Kobayashi-Maskawa matrix is discussed.

  2. Changes in the mean square charge radii and electromagnetic moments of neutron-deficient Bi isotopes

    NASA Astrophysics Data System (ADS)

    Barzakh, A. E.; Batist, L. Kh.; Fedorov, D. V.; Ivanov, V. S.; Molkanov, P. L.; Moroz, F. V.; Orlov, S. Yu.; Panteleev, V. N.; Seliverstov, M. D.; Volkov, Yu. M.

    2015-10-01

    In-source laser spectroscopy experiments for neutron deficient bismuth isotopes at the 306.77 nm atomic transition were carried out at the IRIS (Investigation of Radioactive Isotopes on Synchrocyclotron) facility of Petersburg Nuclear Physics Institute (PNPI). New data on isotope shifts and hyperfine structure for 189-198, 211Bi isotopes and isomers were obtained. The changes in the mean-square charge radii and the magnetic moment values were deduced. Marked deviation from the nearly spherical behavior for ground states of bismuth isotopes at N < 109 is demonstrated, in contrast to the lead and thallium isotopic chains. The big isomer shift between I = 1/2 (intruder) and I = 9/2 (normal) states for odd Bi isotopes (A = 193, 195, 197) was found.

  3. {alpha}-decay properties of the new neutron deficient isotope {sup 212}Pa

    SciTech Connect

    Mitsuoka, S.; Ikezoe, H.; Ikuta, T.; Nagame, Y.; Tsukada, K.; Nishinaka, I.; Oura, Y.; Zhao, Y.L.

    1997-03-01

    The new neutron deficient isotope {sup 212}Pa has been produced in the {sup 182}W({sup 35}Cl,5n) reaction at a beam energy of 182.5 MeV. Evaporation residues have been separated with the JAERI recoil mass separator and identified on the basis of time- and position-correlated {alpha}-decay chains. The {alpha} decay from the ground state of {sup 212}Pa has been observed with an {alpha}-particle energy of 8.270(30) MeV and a half-life of 5.1{sub {minus}1.9}{sup +6.1} ms. {copyright} {ital 1997} {ital The American Physical Society}

  4. {beta}-decay in neutron-deficient Hg, Pb, and Po isotopes

    SciTech Connect

    Moreno, O.; Sarriguren, P.; Alvarez-Rodriguez, R.; Guerra, E. Moya de

    2006-05-15

    The effect of nuclear deformation on the energy distributions of the Gamow-Teller strength is studied in neutron-deficient Hg, Pb, and Po even isotopes. The theoretical framework is based on a self-consistent deformed Skyrme Hartree-Fock mean field with pairing correlations between like nucleons in BCS approximation and residual spin-isospin interactions treated in the proton-neutron quasiparticle random-phase approximation. After a systematic study of the Gamow-Teller strength distributions in the low-excitation-energy region, relevant for {beta}{sup +} decay, we have identified the best candidates to look for deformation signatures in their {beta}{sup +}-decay patterns. {beta}{sup +} half-lives and total Gamow-Teller strengths B(GT{sup {+-}}) are analyzed as well.

  5. Changes in the mean square charge radii and electromagnetic moments of neutron-deficient Bi isotopes

    SciTech Connect

    Barzakh, A. E. Batist, L. Kh.; Fedorov, D. V.; Ivanov, V. S.; Molkanov, P. L.; Moroz, F. V.; Orlov, S. Yu.; Panteleev, V. N.; Seliverstov, M. D.; Volkov, Yu. M.

    2015-10-15

    In-source laser spectroscopy experiments for neutron deficient bismuth isotopes at the 306.77 nm atomic transition were carried out at the IRIS (Investigation of Radioactive Isotopes on Synchrocyclotron) facility of Petersburg Nuclear Physics Institute (PNPI). New data on isotope shifts and hyperfine structure for {sup 189–198,} {sup 211}Bi isotopes and isomers were obtained. The changes in the mean-square charge radii and the magnetic moment values were deduced. Marked deviation from the nearly spherical behavior for ground states of bismuth isotopes at N < 109 is demonstrated, in contrast to the lead and thallium isotopic chains. The big isomer shift between I = 1/2 (intruder) and I = 9/2 (normal) states for odd Bi isotopes (A = 193, 195, 197) was found.

  6. Developing role of short-lived radionuclides in nuclear medical practice. DOE symposium series; 56

    SciTech Connect

    Paras, P.; Thiessen, J.W.

    1985-01-01

    The purpose was to define the developing role and state-of-the-art development of short-lived radionuclides (SLR's) in current nuclear medical practice. Special emphasis was placed on radionuclides with general-purpose labeling capabilities. The need for high-purity labeling-grade iodine-123 was emphasized in the program. Papers have been separately abstracted for the data base. (ACR)

  7. First experimental results of a cryogenic stopping cell with short-lived, heavy uranium fragments produced at 1000 MeV/u

    NASA Astrophysics Data System (ADS)

    Purushothaman, S.; Reiter, M. P.; Haettner, E.; Dendooven, P.; Dickel, T.; Geissel, H.; Ebert, J.; Jesch, C.; Plass, W. R.; Ranjan, M.; Weick, H.; Amjad, F.; Ayet, S.; Diwisch, M.; Estrade, A.; Farinon, F.; Greiner, F.; Kalantar-Nayestanaki, N.; Knöbel, R.; Kurcewicz, J.; Lang, J.; Moore, I. D.; Mukha, I.; Nociforo, C.; Petrick, M.; Pfützner, M.; Pietri, S.; Prochazka, A.; Rink, A.-K.; Rinta-Antila, S.; Scheidenberger, C.; Takechi, M.; Tanaka, Y. K.; Winfield, J. S.; Yavor, M. I.

    2013-11-01

    A cryogenic stopping cell (CSC) has been commissioned with 238U projectile fragments produced at 1000 MeV/u. The spatial isotopic separation in flight was performed with the FRS applying a monoenergetic degrader. For the first time, a stopping cell was operated with exotic nuclei at cryogenic temperatures (70 to 100 K). A helium stopping gas density of up to 0.05\\ \\text{mg/cm}^3 was used, about two times higher than reached before for a stopping cell with RF ion repelling structures. An overall efficiency of up to 15%, a combined ion survival and extraction efficiency of about 50%, and extraction times of 24 ms were achieved for heavy α-decaying uranium fragments. Mass spectrometry with a multiple-reflection time-of-flight mass spectrometer has demonstrated the excellent cleanliness of the CSC. This setup has opened a new field for the spectroscopy of short-lived nuclei.

  8. Spectroscopic factors and cluster decay half-lives of heavy nuclei

    SciTech Connect

    Kuklin, S.N.; Adamian, G.G.; Antonenko, N.V.

    2005-01-01

    The cluster radioactivity is treated under the assumption that the light clusters are produced by a collective motion of the nuclear system in the charge asymmetry coordinate with further penetration through the Coulomb barrier. The known experimental data on cluster radioactivity are described. The half-lives of cluster emission of neutron-deficient actinides and medium-mass nuclei are predicted.

  9. Comparison of short-lived medical isotopes activation by laser thin target induced protons and conventional cyclotron proton beams

    NASA Astrophysics Data System (ADS)

    Murray, Joseph; Dudnikova, Galina; Liu, Tung-Chang; Papadopoulos, Dennis; Sagdeev, Roald; Su, J. J.; UMD MicroPET Team

    2014-10-01

    Production diagnostic or therapeutic nuclear medicines are either by nuclear reactors or by ion accelerators. In general, diagnostic nuclear radioisotopes have a very short half-life varying from tens of minutes for PET tracers and few hours for SPECT tracers. Thus supplies of PET and SPECT radiotracers are limited by regional production facilities. For example 18F-fluorodeoxyglucose (FDG) is the most desired tracer for positron emission tomography because its 110 minutes half-life is sufficient long for transport from production facilities to nearby users. From nuclear activation to completing image taking must be done within 4 hours. Decentralized production of diagnostic radioisotopes will be idea to make high specific activity radiotracers available to researches and clinicians. 11 C, 13 N, 15 O and 18 F can be produced in the energy range from 10-20 MeV by protons. Protons of energies up to tens of MeV generated by intense laser interacting with hydrogen containing targets have been demonstrated by many groups in the past decade. We use 2D PIC code for proton acceleration, Geant4 Monte Carlo code for nuclei activation to compare the yields and specific activities of short-lived isotopes produced by cyclotron proton beams and laser driven protons.

  10. Atomic mass measurements of short-lived nuclides around the doubly-magic 208Pb

    NASA Astrophysics Data System (ADS)

    Weber, C.; Audi, G.; Beck, D.; Blaum, K.; Bollen, G.; Herfurth, F.; Kellerbauer, A.; Kluge, H.-J.; Lunney, D.; Schwarz, S.

    2008-04-01

    Accurate atomic mass measurements of neutron-deficient and neutron-rich nuclides around the doubly-magic 208Pb and of neutron-rich cesium isotopes were performed with the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The masses of 145,147Cs, 181,183Tl, 186Tl m, 187Tl m, 196Tl m, 205Tl, 197Pb m, 208Pb, 190-197Bi, 209,215,216Bi, 203,205,229Fr, and 214,229,230Ra were determined. The obtained relative mass uncertainty in the range of 2×10 to 2×10 is not only required for safe identification of isomeric states but also allows mapping the detailed structure of the mass surface. A mass adjustment procedure was carried out and the results included into the Atomic Mass Evaluation. The resulting separation energies are discussed and the mass spectrometric and laser spectroscopic data are examined for possible correlations.

  11. Charge radii and nuclear moments of neutron-deficient potassium isotopes

    NASA Astrophysics Data System (ADS)

    Minamisono, K.; Barquest, B. R.; Bollen, G.; Hughes, M.; Strum, R.; Tarazona, D.; Asberry, H. B.; Cooper, K.; Hammerton, K.; Klose, A.; Mantica, P. F.; Morrissey, D. J.; Geppert, Ch.; Harris, J.; Ringle, R.; Rodriguez, J. A.; Rossi, D. M.; Ryder, C. A.; Smith, A.; Schwarz, S.; Sumithrarachchi, C.

    2014-09-01

    The monotonic change of charge radii of K isotopes across N = 20 suggests a reduction of the shell gap. A systematic study of the charge radii and ground state magnetic and quadrupole moments of neutron-deficient 35-37K isotopes is underway at the BEam COoling and LAser spectroscopy (BECOLA) facility at NSCL/MSU to investigate the anomalous trend in charge radii. The K isotopes were produced by fragmentation of a 40Ca beam, thermalized in a linear gas cell, extracted at an energy of 30 keV, and transported to BECOLA. The K ion beam was cooled and bunched, and neutralized in a Na vapor cell. Laser-induced fluorescence was detected as a function of the Doppler-tuned laser frequency and time relative to the release of the beam bunch. The beta-NMR technique was used to determine ground-state nuclear moments, where hyperfine splittings are too small to resolve using collinear laser spectroscopy. The monotonic change of charge radii of K isotopes across N = 20 suggests a reduction of the shell gap. A systematic study of the charge radii and ground state magnetic and quadrupole moments of neutron-deficient 35-37K isotopes is underway at the BEam COoling and LAser spectroscopy (BECOLA) facility at NSCL/MSU to investigate the anomalous trend in charge radii. The K isotopes were produced by fragmentation of a 40Ca beam, thermalized in a linear gas cell, extracted at an energy of 30 keV, and transported to BECOLA. The K ion beam was cooled and bunched, and neutralized in a Na vapor cell. Laser-induced fluorescence was detected as a function of the Doppler-tuned laser frequency and time relative to the release of the beam bunch. The beta-NMR technique was used to determine ground-state nuclear moments, where hyperfine splittings are too small to resolve using collinear laser spectroscopy. This work was supported in part by NSF Grant No. PHY-11-02511.

  12. Experimental Measurements of Short-Lived Fission Products from Uranium, Neptunium, Plutonium and Americium

    SciTech Connect

    Metz, Lori A.; Payne, Rosara F.; Friese, Judah I.; Greenwood, Lawrence R.; Kephart, Jeremy D.; Pierson, Bruce D.

    2009-11-01

    Fission yields are especially well characterized for long-lived fission products. Modeling techniques incorporate numerous assumptions and can be used to deduce information about the distribution of short-lived fission products. This work is an attempt to gather experimental (model-independent) data on the short-lived fission products. Fissile isotopes of uranium, neptunium, plutonium and americium were irradiated under pulse conditions at the Washington State University 1 MW TRIGA reactor to achieve ~108 fissions. The samples were placed on a HPGe (high purity germanium) detector to begin counting in less than 3 minutes post irradiation. The samples were counted for various time intervals ranging from 5 minutes to 1 hour. The data was then analyzed to determine which radionuclides could be quantified and compared to the published fission yield data.

  13. Emission Channeling with Short-Lived Isotopes (EC-SLI) at CERN's ISOLDE Facility

    NASA Astrophysics Data System (ADS)

    Wahl, U.; Correia, J. G.; Costa, A.; David-Bosne, E.; Pereira, L. M. C.; Amorim, L. M.; Augustyns, V.; Temst, K.; Vantomme, A.; da Silva, M. R.; Silva, D. J.; Araújo, J. P.; Miranda, P.; Bharuth-Ram, K.

    2015-11-01

    We give an overview on the historical development and current program for lattice location studies at CERN's ISOLDE facility, where the EC-SLI (Emission Channeling with Short-Lived Isotopes) collaboration maintains several setups for this type of experiments. We illustrate that the three most decisive factors for the success of the technique are access to facilities producing radioactive isotopes, position-sensitive detectors for the emitted decay particles, and reliable simulation codes which allow for quantitative analysis.

  14. Deformation studies in the extremely neutron-deficient praseodymium, neodymium and promethium isotopes

    SciTech Connect

    Breitenbach, J.; Braga, R.A.; Wood, J.L. ); Semmes, P.B. . Dept. of Physics); Kormicki, J. . Dept. of Physics)

    1992-01-01

    Several experiments were performed at the UNISOR isotope separator facility at HHIRF at the Oak Ridge National Laboratory on the [beta][sup +]/EC decay of neutron-deficient rare earth isotopes. Data for the three decay chains [sup 137]Eu [yields] [sup 137]Sm [yields] [sup 137]Pm [yields] [sup 137]Nd, [sup 135]Sm [yields] [sup 135]Pm [yields] [sup 135]Nd and [sup 133]Sm [yields] [sup 133]Pm [yields] [sup 133]Nd were obtained consisting of multiscaled spectra of [gamma] rays, x rays, and conversion electrons, as well as [gamma][gamma]t, X[gamma]t, e[gamma]t and eXt coincidences. Gamma rays associated with the decay of [sup 133]Sm and [sup 133]Pm were observed for the first time. The decay of a new low-spin (1/2,3/2) isomeric state, with a half life around 70 sec was seen in [sup 133]Nd. Systematics and particle-rotor calculations are discussed.

  15. Deformation studies in the extremely neutron-deficient praseodymium, neodymium and promethium isotopes

    SciTech Connect

    Breitenbach, J.; Braga, R.A.; Wood, J.L.; Semmes, P.B.; Kormicki, J.

    1992-12-31

    Several experiments were performed at the UNISOR isotope separator facility at HHIRF at the Oak Ridge National Laboratory on the {beta}{sup +}/EC decay of neutron-deficient rare earth isotopes. Data for the three decay chains {sup 137}Eu {yields} {sup 137}Sm {yields} {sup 137}Pm {yields} {sup 137}Nd, {sup 135}Sm {yields} {sup 135}Pm {yields} {sup 135}Nd and {sup 133}Sm {yields} {sup 133}Pm {yields} {sup 133}Nd were obtained consisting of multiscaled spectra of {gamma} rays, x rays, and conversion electrons, as well as {gamma}{gamma}t, X{gamma}t, e{gamma}t and eXt coincidences. Gamma rays associated with the decay of {sup 133}Sm and {sup 133}Pm were observed for the first time. The decay of a new low-spin (1/2,3/2) isomeric state, with a half life around 70 sec was seen in {sup 133}Nd. Systematics and particle-rotor calculations are discussed.

  16. Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes

    NASA Astrophysics Data System (ADS)

    Kesteloot, N.; Bastin, B.; Gaffney, L. P.; Wrzosek-Lipska, K.; Auranen, K.; Bauer, C.; Bender, M.; Bildstein, V.; Blazhev, A.; Bönig, S.; Bree, N.; Clément, E.; Cocolios, T. E.; Damyanova, A.; Darby, I.; De Witte, H.; Di Julio, D.; Diriken, J.; Fransen, C.; García-Ramos, J. E.; Gernhäuser, R.; Grahn, T.; Heenen, P.-H.; Hess, H.; Heyde, K.; Huyse, M.; Iwanicki, J.; Jakobsson, U.; Konki, J.; Kröll, T.; Laurent, B.; Lecesne, N.; Lutter, R.; Pakarinen, J.; Peura, P.; Piselli, E.; Próchniak, L.; Rahkila, P.; Rapisarda, E.; Reiter, P.; Scheck, M.; Seidlitz, M.; Sferrazza, M.; Siebeck, B.; Sjodin, M.; Tornqvist, H.; Traykov, E.; Van De Walle, J.; Van Duppen, P.; Vermeulen, M.; Voulot, D.; Warr, N.; Wenander, F.; Wimmer, K.; Zielińska, M.

    2015-11-01

    Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po 196 ,198 ,200 ,202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po,202200, the transitional and diagonal matrix elements of the 21+ state are determined. In Po,198196 multistep Coulomb excitation is observed, populating the 41+,02+ , and 22+ states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from 196Po onwards. Three model descriptions are used to compare to the data. Calculations with the beyond-mean-field model, the interacting boson model, and the general Bohr Hamiltonian model show partial agreement with the experimental data. Finally, calculations with a phenomenological two-level mixing model hint at the mixing of a spherical structure with a weakly deformed rotational structure.

  17. Classification of short-lived objects using an interactive adaptable assistance system

    NASA Astrophysics Data System (ADS)

    El Bekri, Nadia; Angele, Susanne; Peinsipp-Byma, Elisabeth

    2015-05-01

    "Although we know that it is not a familiar object, after a while we can say what it resembles". The core task of an aerial image analyst is to recognize different object types based on certain clearly classified characteristics from aerial or satellite images. An interactive recognition assistance system compares selected features with a fixed set of reference objects (core data set). Therefore it is mainly designed to evaluate durable single objects like a specific type of ship or vehicle. Aerial image analysts on missions realized a changed warfare over the time. The task was not anymore to classify and thereby recognize a single durable object. The problem was that they had to classify strong variable objects and the reference set did not match anymore. In order to approach this new scope we introduce a concept to a further development of the interactive assistance system to be able to handle also short-lived, not clearly classifiable and strong variable objects like for example dhows. Dhows are the type of ships that are often used during pirate attacks at the coast of West Africa. Often these ships were build or extended by the pirates themselves. They follow no particular pattern as the standard construction of a merchant ship. In this work we differ between short-lived and durable objects. The interactive adaptable assistance system is supposed to assist image analysts with the classification of objects, which are new and not listed in the reference set of objects yet. The human interaction and perception is an important factor in order to realize this task and achieve the goal of recognition. Therefore we had to model the possibility to classify short-lived objects with appropriate procedures taking into consideration all aspects of short-lived objects. In this paper we will outline suitable measures and the possibilities to categorize short-lived objects via simple basic shapes as well as a temporary data storage concept for shortlived objects. The

  18. Neutron-deficient N{approx_equal}126 nuclei produced in 238U fragmentation: population of high-spin states

    SciTech Connect

    Podolyak, Zs.; Regan, P. H.; Walker, P. M.; Pearson, C. J.; Valiente-Dobon, J. J.; Gerl, J.; Hellstroem, M.; Becker, F.; Gorska, M.; Kelic, A.; Kopatch, Y.; Mandal, S.; Schmidt, K.-H.; Wollersheim, H. J.; Banu, A.; Geissel, H.; Grawe, H.; Kojouharov, I.; Lozeva, R.; Portillo, M.

    2006-04-26

    The population of metastable states produced in relativistic-energy fragmentation of a 238U beam has been measured. For states with high angular momentum, I=17({Dirac_h}/2{pi}) and I=21.5({Dirac_h}/2{pi}), a higher population than expected has been observed, with the discrepancy increasing with angular momentum. By considering two sources for the angular momentum, related to single-particle and collective motions, a much improved description of the experimental results can be obtained. In addition, new results on the structure of 208Fr, 211Ra and 216Ac are reported.

  19. Very elongated nuclei near A = 194

    SciTech Connect

    Becker, J.A.; Henry, E.A.; Yates, S.W.; Wang, T.F.; Kuhnert, A. ); Brinkman, M.J.; Cizewski, J.A. ); Deleplanque, M.A.; Diamond, R.M.; Stephens, F.S.; Azaiez, F.; Korten, W.; Draper, J.E. )

    1990-10-01

    A {gamma}-ray cascade in {sup 191}Hg of 12 members with average energy spacing 37 keV and Q{sub t} {equals} 18(3)eb was reported by Moore, and coworkers in 1989. This was the first report of very elongated nuclei (superdeformation) in this mass region. Since then, some 25 {gamma}-ray cascades have been observed in 11 (slightly neutron deficient) Hg, Pb and Tl nuclei. The bands have similar dynamic moments-of-inertia. Some nuclei exhibit multiple bands, and the backbending phenomena has been observed. Level spins can be obtained from comparison of transition energies to rotational model formulas. Selected bands (in different nuclei) have equal transition energies (within 0.1%). Alignment in integer multiples of {h bar} has been observed. Properties of these bands will be described. 27 refs., 3 figs.

  20. Charge radii of neutron-deficient 36K and 37K

    NASA Astrophysics Data System (ADS)

    Rossi, D. M.; Minamisono, K.; Asberry, H. B.; Bollen, G.; Brown, B. A.; Cooper, K.; Isherwood, B.; Mantica, P. F.; Miller, A.; Morrissey, D. J.; Ringle, R.; Rodriguez, J. A.; Ryder, C. A.; Smith, A.; Strum, R.; Sumithrarachchi, C.

    2015-07-01

    Background: The systematic trend in mean-square charge radii as a function of proton or neutron number exhibits a discontinuity at the nucleon-shell closures. While the established N =28 shell closure is evident in the charge radii of the isotopic chains of K through Mn, a similar signature of the N =20 shell closure is absent in the Ca region. Purpose: The isotope shift between neutron-deficient 36K and 37K was determined to investigate the change of the mean-square charge radii across N =20 in the K isotopic chain. Methods: The D 1 atomic hyperfine spectra of 36K and 37K were measured using an optical pumping and subsequent β -decay asymmetry detection technique. Atomic rate equations were solved to fit the resonant line shape. The result was compared to Skyrme energy-density functional and shell-model calculations. Results: The isotope shift was obtained as δ ν37 ,36=-139 (4 ) (3 ) MHz. Using a re-evaluated isotope shift, δ ν39 ,37=-264 (2 ) (3 ) MHz, the isotope shift relative to 39K was determined to be δ ν39 ,36=-403 (5 ) (4 ) MHz. The differential mean-square charge radius was then deduced as δ 39 ,36=-0.16 (5 ) (8 ) fm2 . The Skyrme energy-density functional and shell-model calculations overpredict the experimental values below N =20 and underpredict them above N =20 , and their agreement is marginal. Conclusions: The absence of the shell-closure signature at N =20 in the K isotopic chain is understood as a balance between the monopole and the quadrupole proton-core polarizations below and above N =20 , respectively.

  1. Have we underestimated the role of short-lived chlorine compounds in ozone depletion?

    NASA Astrophysics Data System (ADS)

    Oram, David; Laube, Johannes; Sturges, Bill; Gooch, Lauren; Leedham, Emma; Ashfold, Matthew; Pyle, John; Abu Samah, Azizan; Moi Phang, Siew; Ou-Yang, Chang-Feng; Lin, Neng-Huei; Wang, Jia-Lin; Brenninkmeijer, Carl

    2015-04-01

    In recent years much attention has been focussed on the potential of bromine-containing VSLS (very short lived substances) to contribute to stratospheric ozone depletion. This is primarily due to the large observed discrepancy between the measured inorganic bromine in the stratosphere and the amount of bromine available from known, longer lived sources gases (halons and CH3Br). In contrast, the role of very short-lived chlorine compounds (VSLS-CL) has been considered trivial because they contribute only a few percent to the total organic chlorine in the troposphere, the majority of which is supplied by long-lived compounds such as the CFCs, HCFCs, methyl chloroform and carbon tetrachloride. However recent evidence shows that one VSLS-Cl, dichloromethane (CH2Cl2) has increased by 60% over the past decade (WMO, 2014) and has already begun to offset the long-term decline in stratospheric chlorine loading caused by the reduction in emissions of substances controlled by the Montreal Protocol. We will present new VSLS-Cl measurements from recent ground-based and aircraft campaigns in SE Asia where we have observed dramatic enhancements in a number of VSLS-Cl, including CH2Cl2. Furthermore we will demonstrate how pollution from China and the surrounding region can rapidly, and regularly, be transported across the South China Sea and subsequently uplifted to altitudes of 11-12 km, the region close to the lower TTL. This process occurs frequently during the winter monsoon season and could represent a fast and efficient mechanism for transporting short-lived compounds, and other pollutants, to the lower stratosphere.

  2. ``Sleeping reactor`` irradiations: Shutdown reactor determination of short-lived activation products

    SciTech Connect

    Jerde, E.A.; Glasgow, D.C.

    1998-09-01

    At the High-Flux Isotope Reactor (HFIR) at the Oak Ridge National Laboratory, the principal irradiation system has a thermal neutron flux ({phi}) of {approximately} 4 {times} 10{sup 14} n/cm{sup 2} {center_dot} s, permitting the detection of elements via irradiation of 60 s or less. Irradiations of 6 or 7 s are acceptable for detection of elements with half-lives of as little as 30 min. However, important elements such as Al, Mg, Ti, and V have half-lives of only a few minutes. At HFIR, these can be determined with irradiation times of {approximately} 6 s, but the requirement of immediate counting leads to increased exposure to the high activity produced by irradiation in the high flux. In addition, pneumatic system timing uncertainties (about {+-} 0.5 s) make irradiations of < 6 s less reliable. Therefore, the determination of these ultra-short-lived species in mixed matrices has not generally been made at HFIR. The authors have found that very short lived activation products can be produced easily during the period after reactor shutdown (SCRAM), but prior to the removal of spent fuel elements. During this 24- to 36-h period (dubbed the ``sleeping reactor``), neutrons are produced in the beryllium reflector by the reaction {sup 9}Be({gamma},n){sup 8}Be, the gamma rays principally originating in the spent fuel. Upon reactor SCRAM, the flux drops to {approximately} 1 {times} 10{sup 10} n/cm{sup 2} {center_dot} s within 1 h. By the time the fuel elements are removed, the flux has dropped to {approximately} 6 {times} 10{sup 8}. Such fluxes are ideal for the determination of short-lived elements such as Al, Ti, Mg, and V. An important feature of the sleeping reactor is a flux that is not constant.

  3. Absence of replicative senescence in cultured cells from the short-lived killifish Nothobranchius furzeri.

    PubMed

    Graf, Michael; Hartmann, Nils; Reichwald, Kathrin; Englert, Christoph

    2013-01-01

    A major challenge in age research is the absence of short-lived vertebrate model organisms. The turquoise killifish Nothobranchius furzeri has the shortest known lifespan of a vertebrate that can be bred in captivity. The short lived GRZ strain only reaches a maximum age of 3-4 months, whereas other strains (MZM) reach 6-10 months. Most importantly, the short lifespan is associated with typical signs of ageing. To find out more about possible cellular factors that might contribute to the short lifespan and to the difference in lifespan between strains, we analyzed the expression of markers for cellular senescence. Expression of Tp53, Cdkn1a and Cdkn2a/b in skin revealed no change in the short-lived GRZ but increased expression of the cell cycle inhibitors Cdkn1a and Cdkn2a/b in the long-lived MZM strain with age. This suggests that expression of distinct cell cycle inhibitors reflects rather chronological than biological age in N. furzeri. To study the relationship of organismal life span and in vitro life span of cells, we established a primary cell culture model. For both strains we demonstrate here the absence of replicative senescence as analysed by morphology, expression of Cdkn1a and Cdkn2a/b, population doubling times and γH2AFX in long-term and short-term cultured cells. We reason this to be on account of sustained telomerase activity and maintained telomeric length. Hence, we propose that differences in maximum life span of different N. furzeri strains is not reflected by differences in proliferation speed or replicative potential of the respective cultured cells. PMID:22445733

  4. Quantum non-locality in a two-slit interferometer for short-lived particles

    SciTech Connect

    Klein, Spencer R.; Nystrand, Joakim

    2001-12-01

    We describe a new test of quantum nonlocality, using an interferometer for short-lived particles. The separation is large compared with the particle lifetimes. This interferometer is realized by vector meson production in distant heavy ion collisions. The mesons decay before waves from the two sources (ions) can overlap, so interference is only possible among the decay products. The post-decay wave function must retain amplitudes for all possible decays. The decay products are spatially separated, necessitating a non-local wave function. The interference is measurable by summing the product momenta. Alternately, the products positions could be observed, allowing new tests of the EPR paradox.

  5. An effective technique for the storage of short lived radioactive gaseous waste.

    PubMed

    Schweiger, Lutz

    2011-09-01

    An effective technique is described to deal with volatile, short lived radioactive waste generated as a result of the routinely produced positron emission tomography (PET) radiopharmaceutical 2-deoxy-2-[(18)F]fluoro-D-glucose (FDG). All radioactive gases and aerosols created during the synthesis are collected and stored safely in commercially available TEDLAR gas sampling bags. Once these collected PET by-products decay, the TEDLAR gas bags can be easily emptied and reused. This improved technique is effective, safe, reliable and economical. PMID:21592805

  6. Short-lived positron emitters in beam-on PET imaging during proton therapy

    NASA Astrophysics Data System (ADS)

    Dendooven, P.; Buitenhuis, H. J. T.; Diblen, F.; Heeres, P. N.; Biegun, A. K.; Fiedler, F.; van Goethem, M.-J.; van der Graaf, E. R.; Brandenburg, S.

    2015-12-01

    The only method for in vivo dose delivery verification in proton beam radiotherapy in clinical use today is positron emission tomography (PET) of the positron emitters produced in the patient during irradiation. PET imaging while the beam is on (so called beam-on PET) is an attractive option, providing the largest number of counts, the least biological washout and the fastest feedback. In this implementation, all nuclides, independent of their half-life, will contribute. As a first step towards assessing the relevance of short-lived nuclides (half-life shorter than that of 10C, T1/2  =  19 s) for in vivo dose delivery verification using beam-on PET, we measured their production in the stopping of 55 MeV protons in water, carbon, phosphorus and calcium The most copiously produced short-lived nuclides and their production rates relative to the relevant long-lived nuclides are: 12N (T1/2  =  11 ms) on carbon (9% of 11C), 29P (T1/2  =  4.1 s) on phosphorus (20% of 30P) and 38mK (T1/2  =  0.92 s) on calcium (113% of 38gK). No short-lived nuclides are produced on oxygen. The number of decays integrated from the start of an irradiation as a function of time during the irradiation of PMMA and 4 tissue materials has been determined. For (carbon-rich) adipose tissue, 12N dominates up to 70 s. On bone tissue, 12N dominates over 15O during the first 8-15 s (depending on carbon-to-oxygen ratio). The short-lived nuclides created on phosphorus and calcium provide 2.5 times more beam-on PET counts than the long-lived ones produced on these elements during a 70 s irradiation. From the estimated number of 12N PET counts, we conclude that, for any tissue, 12N PET imaging potentially provides equal to superior proton range information compared to prompt gamma imaging with an optimized knife-edge slit camera. The practical implementation of 12N PET imaging is discussed.

  7. Accurate mass determination of short-lived isotopes by a tandem Penning-trap mass spectrometer

    SciTech Connect

    Stolzenberg, H.; Becker, S.; Bollen, G.; Kern, F.; Kluge, H.; Otto, T.; Savard, G.; Schweikhard, L. ); Audi, G. ); Moore, R.B. ); The ISOLDE Collaboration

    1990-12-17

    A mass spectrometer consisting of two Penning traps has been set up for short-lived isotopes at the on-line mass separator ISOLDE at CERN. The ion beam is collected and cooled in the first trap. After delivery to the second trap, high-accuracy direct mass measurements are made by determining the cyclotron frequency of the stored ions. Measurements have been performed for {sup 118}Cs--{sup 137}Cs. A resolving power of over 10{sup 6} and an accuracy of 1.4{times}10{sup {minus}7} have been achieved, corresponding to about 20 keV.

  8. Inducible transgenic expression in the short-lived fish Nothobranchius furzeri.

    PubMed

    Allard, J B; Kamei, H; Duan, C

    2013-05-01

    This study demonstrates inducible transgenic expression in the exceptionally short-lived turquoise killifish Nothobranchius furzeri, which is a useful vertebrate model for ageing research. Transgenic N. furzeri bearing a green fluorescent protein (Gfp) containing construct under the control of a heat shock protein 70 promoter were generated, heat shock-induced and reversible Gfp expression was demonstrated and germline transmission of the transgene to the F1 and F2 generations was achieved. The availability of this inducible transgenic expression system will make the study of ageing-related antagonistically pleiotropic genes possible using this unique vertebrate model organism. PMID:23639168

  9. Properties of short-living ball lightning produced in the laboratory

    NASA Astrophysics Data System (ADS)

    Egorov, A. I.; Stepanov, S. I.

    2008-06-01

    An experimental setup for highly reproducible generation of artificial ball lightnings is implemented. Thousands of floating glowing plasmoids 12-20 cm in diameter are produced. Research facilities for studying the plasmoids are developed. It is found that short-lived ball lightnings live for about 1 s and carry an electric charge. The lightnings are shown to have a complex structure: a central kernel containing a rich variety of hydrated ions and aerosol of decay products is surrounded by a thin negatively charged shell.

  10. Tantalum-178--a short-lived nuclide for nuclear medicine: development of a potential generator system.

    PubMed

    Neirinckx, R D; Jones, A G; Davis, M A; Harris, G I; Holman, B L

    1978-05-01

    We describe a chemical separation that may form the basis of a generator system for the short-lived radionuclide Ta-178 (T 1/2 = 9 min). The parent nuclide W-178 (T 1/2 = 21.7 days) is loaded on an anion-exchange column and the daughter eluted with a mixture of dilute hydrochloric acid and hydrogen peroxide. The yields of tantalum and the breakthrough of the tungsten parent as a function of the eluting conditions are discussed, and preliminary animal distribution data are presented for various treatments of the eluant solution. PMID:641574

  11. PTF10iya: a short-lived, luminous flare from the nuclear region of a star-forming galaxy

    NASA Astrophysics Data System (ADS)

    Cenko, S. Bradley; Bloom, Joshua S.; Kulkarni, S. R.; Strubbe, Linda E.; Miller, Adam A.; Butler, Nathaniel R.; Quimby, Robert M.; Gal-Yam, Avishay; Ofek, Eran O.; Quataert, Eliot; Bildsten, Lars; Poznanski, Dovi; Perley, Daniel A.; Morgan, Adam N.; Filippenko, Alexei V.; Frail, Dale A.; Arcavi, Iair; Ben-Ami, Sagi; Cucchiara, Antonio; Fassnacht, Christopher D.; Green, Yoav; Hook, Isobel M.; Howell, D. Andrew; Lagattuta, David J.; Law, Nicholas M.; Kasliwal, Mansi M.; Nugent, Peter E.; Silverman, Jeffrey M.; Sullivan, Mark; Tendulkar, Shriharsh P.; Yaron, Ofer

    2012-03-01

    We present the discovery and characterization of PTF10iya, a short-lived (Δt≈ 10 d, with an optical decay rate of ˜0.3 mag d-1), luminous (? mag) transient source found by the Palomar Transient Factory. The ultraviolet/optical spectral energy distribution is reasonably well fitted by a blackbody with T≈ (1-2) × 104 K and peak bolometric luminosity LBB≈ (1-5) × 1044 erg s-1 (depending on the details of the extinction correction). A comparable amount of energy is radiated in the X-ray band that appears to result from a distinct physical process. The location of PTF10iya is consistent with the nucleus of a star-forming galaxy (z= 0.224 05 ± 0.000 06) to within 350 mas (99.7 per cent confidence radius), or a projected distance of less than 1.2 kpc. At first glance, these properties appear reminiscent of the characteristic 'big blue bump' seen in the near-ultraviolet spectra of many active galactic nuclei (AGNs). However, emission-line diagnostics of the host galaxy, along with a historical light curve extending back to 2007, show no evidence for AGN-like activity. We therefore consider whether the tidal disruption of a star by an otherwise quiescent supermassive black hole may account for our observations. Though with limited temporal information, PTF10iya appears broadly consistent with the predictions for the early 'super-Eddington' phase of a solar-type star being disrupted by a ˜107 M⊙ black hole. Regardless of the precise physical origin of the accreting material, the large luminosity and short duration suggest that otherwise quiescent galaxies can transition extremely rapidly to radiate near the Eddington limit; many such outbursts may have been missed by previous surveys lacking sufficient cadence.

  12. Al-26 and Be-10 in Efremovka and Acfer CAIs: Constraints on the Origin of Short-lived Radionuclides

    NASA Astrophysics Data System (ADS)

    Srinivasan, G.; Chaussidon, M.; Bischoff, A.

    2007-03-01

    In this abstract we present aluminum-26 and beryllium-10 abundances in Efremovka and Acfer CAIs. These measurements help us to constrain the origin of short-lived radionuclides aluminum-26, beryllium-10.

  13. Shape Coexistence in Pb-Rn Nuclei Studied by Particle Decay Spectroscopy

    NASA Astrophysics Data System (ADS)

    Andreyev, A. N.

    2006-08-01

    This contribution reviews the results of recent experiments at the velocity filter SHIP (GSI, Darmstadt) in which a number of very neutron-deficient nuclei with Z=83-88 and N< 126 were studied in detail and new nuclides 186,187Po, 192At and 193,194Rn were identified. Complete fusion reactions at beam energies close to the Coulomb barrier were used, followed by particle detection with various detection systems. Peculiarities in α-decay characteristics of the 186-191Po isotopes are discussed in detail. Very recent results for the neutron-deficient At-Ra nuclei from the gas-filled separator RITU (JYFL, Jyväskylä) are also highlighted. The application of a new method to reach nuclei in this region — spallation-evaporation reactions of 238U ions at 1 AGeV on a Be target, followed by the separation with the FRS at GSI is discussed as well.

  14. Shape Coexistence in Pb-Rn Nuclei Studied by Particle Decay Spectroscopy

    SciTech Connect

    Andreyev, A. N.

    2006-08-14

    This contribution reviews the results of recent experiments at the velocity filter SHIP (GSI, Darmstadt) in which a number of very neutron-deficient nuclei with Z=83-88 and N< 126 were studied in detail and new nuclides 186,187Po, 192At and 193,194Rn were identified. Complete fusion reactions at beam energies close to the Coulomb barrier were used, followed by particle detection with various detection systems. Peculiarities in {alpha}-decay characteristics of the 186-191Po isotopes are discussed in detail. Very recent results for the neutron-deficient At-Ra nuclei from the gas-filled separator RITU (JYFL, Jyvaeskylae) are also highlighted.The application of a new method to reach nuclei in this region - spallation-evaporation reactions of 238U ions at 1 AGeV on a Be target, followed by the separation with the FRS at GSI is discussed as well.

  15. Universal Slow RI-Beam Facility at RIKEN RIBF for Laser Spectroscopy of Short-Lived Nuclei

    SciTech Connect

    Wada, M.; Takamine, A.; Okada, K.; Sonoda, T.; Schury, P.; Kanai, Y.; Kojima, T. M.; Lioubimov, V.; Yamazaki, Y.; Yoshida, A.; Kubo, T.; Iimura, H.; Katayama, I.; Ohtani, S.; Wollnik, H.; Schuessler, H. A.

    2009-03-17

    A universal slow RI-beam facility (SLOWRI) for precision atomic spectroscopy is being built at the RIKEN RI-beam factory. The facility will provide a wide variety of low-energy nuclear ions of all elements produced by projectile fragmentation of high-energy heavy-ion beams and thermalized by an RF-carpet ion guide. At prototype SLOWRI, radioactive Be isotope ions produced at 1 GeV were decelerated and cooled in an ion trap down to 1 {mu}eV by employing laser cooling. The ground state hyperfine structures of {sup 7}Be{sup +} and {sup 11}Be{sup +} were measured accurately by laser microwave double resonance spectroscopy. Measurements of the S{sub 1/2}{yields}P{sub 1/2}, P{sub 3/2} transition frequencies of {sup 7,9,10,11}Be{sup +} ions are also in progress aiming at the study of the nuclear charge radii. Other possible experiment at SLOWRI, such as mass spectroscopy, are also discussed.

  16. Very short-lived and stable mRNAs from resting human lymphocytes.

    PubMed Central

    Berger, S L; Cooper, H L

    1975-01-01

    The kinetics of degradation of newly synthesized cytoplasmic poly(A)-bearing RNA have been examined in resting human lymphocytes. Two classes were identified, a very labile component with a half-life of less than 17 min and a stable component which remains apparently undiminished during 24 hr of observation. Both classes have molecular weights between 2.5 and 3.5 x 10(5) but the stable material has a narrower size distribution and a slightly lower average molecular weight than the short-lived component. The fate of stable RNA synthesized in the resting cell was also examined after growth stimulation with phytohemagglutinin after 2 and 6 hr of treatment. No transfer of stable material into the labile pool could be discerned; the amount of stable material remained constant. The existence of two species of mRNAs with different lifetimes in animal cells provides a potential means for regulation of protein synthesis by controlling the supply of specific messages. Furthermore, such a short-lived mRNA species may explain the observed disparity between the amount of poly(A)-bearing heterogeneous RNA produced in the nucleus and the amount of mature message found in the cytoplasm. PMID:1060069

  17. Transition from long- to short-lived transient pores in giant vesicles in an aqueous medium

    NASA Astrophysics Data System (ADS)

    Rodriguez, Nicolas; Cribier, Sophie; Pincet, Frédéric

    2006-12-01

    We have observed large pores in the membrane of giant vesicles in an aqueous medium. The lifetime of the pores can reach 2min and their size (a few micrometers) enables their visualization by fluorescence microscopy. These pores are obtained thanks to a destabilization of the membrane due to the synergistic action of a cone-shaped and nitrobenzodiazole (NBD) labeled phospholipid illuminated in the presence of dithionite. The opening of the pore occurs immediately after illumination starts so that it can be accurately triggered. A concomitant decrease of the vesicle radius is observed; we interpret it as a solubilization of the membrane. Depending on the rate of this solubilization, long- or short-lived pores were observed. At the transition between both regimes for a 30μm vesicle, the solubilization rate was about 1/300s-1 . In order to interpret these observations, we have revisited the current model of pore opening to take into account this solubilization. This proposed model along with simulations enables us to prove that solubilization explains why the large long-lived pores are observed even in an aqueous medium. The model also predicts the solubilization rate at the transition between a single long-lived pore and a cascade of short-lived pores.

  18. Short-lived pollutants in the Arctic: their climate impact and possible mitigation strategies

    SciTech Connect

    Menon, Surabi; Quinn, P.K.; Bates, T.S.; Baum, E.; Doubleday, N.; Fiore, A.M.; Flanner, M.; Fridlind, A.; Garrett, T.J.; Koch, D.; Menon, S.; Shindell, D.; Stohl, A.; Warren, S.G.

    2007-09-24

    Several short-lived pollutants known to impact Arctic climate may be contributing to the accelerated rates of warming observed in this region relative to the global annually averaged temperature increase. Here, we present a summary of the short-lived pollutants that impact Arctic climate including methane, tropospheric ozone, and tropospheric aerosols. For each pollutant, we provide a description of the major sources and the mechanism of forcing. We also provide the first seasonally averaged forcing and corresponding temperature response estimates focused specifically on the Arctic. The calculations indicate that the forcings due to black carbon, methane, and tropospheric ozone lead to a positive surface temperature response indicating the need to reduce emissions of these species within and outside the Arctic. Additional aerosol species may also lead to surface warming if the aerosol is coincident with thin, low lying clouds. We suggest strategies for reducing the warming based on current knowledge and discuss directions for future research to address the large remaining uncertainties.

  19. Evolution of nuclear ground-state properties of neutron-deficient isotopes around Z =82 from precision mass measurements

    NASA Astrophysics Data System (ADS)

    Böhm, Ch.; Borgmann, Ch.; Audi, G.; Beck, D.; Blaum, K.; Breitenfeldt, M.; Cakirli, R. B.; Cocolios, T. E.; Eliseev, S.; George, S.; Herfurth, F.; Herlert, A.; Kowalska, M.; Kreim, S.; Lunney, D.; Manea, V.; Minaya Ramirez, E.; Naimi, S.; Neidherr, D.; Rosenbusch, M.; Schweikhard, L.; Stanja, J.; Wang, M.; Wolf, R. N.; Zuber, K.

    2014-10-01

    High-precision mass measurements of neutron-deficient Tl (A =184, 186, 190, 193-195, 198) isotopes as well as Pb (A =202,208), Fr (A =207,208), and Ra (A =224) are performed with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The improved precision of the mass data now allows the study of subtle odd-even effects. The gradual development of collectivity with the removal of protons from the magic Z =82 core is analyzed by combining the new mass results with nuclear charge-radii data and mean-field model predictions.

  20. Exotic modes of excitation in proton rich nuclei

    SciTech Connect

    Paar, N.

    2011-11-30

    The framework of relativistic energy density functional has been applied in description of excitation phenomena in nuclei close to the proton drip line. In particular, low-lying dipole excitations have been studied using relativistic quasiparticle random phase approximation, based on effective Lagrangians with density dependent meson nucleon couplings. In the isovector dipole channel, the occurrence of pronounced low-lying dipole peaks is predicted, corresponding to the proton pygmy dipole resonance. Since this exotic mode still awaits its experimental confirmation, systematic calculations have been conducted within a pool of neutron deficient nuclei, in order to identify the best possible candidates for measurements.

  1. Implicit short-lived motor representations of space in brain damaged and healthy subjects.

    PubMed

    Rossetti, Y

    1998-09-01

    This article reviews experimental evidence for a specific sensorimotor function which can be dissociated from higher level representations of space. It attempts to delineate this function on the basis of results obtained by psychophysical experiments performed with brain damaged and healthy subjects. Eye and hand movement control exhibit automatic features, such that they are incompatible with conscious control. In addition, they rely on a reference frame different from the one used by conscious perception. Neuropsychological cases provide a strong support for this specific motor representation of space, which can be spared in patients with lesions of primary sensory systems who have lost conscious perception of visual, tactile or proprioceptive stimuli. Observation of these patients also showed that their motor behavior can be "attracted" by a goal only under specific conditions, that is, when the response is immediate and when no cognitive representation of this goal is elaborated at the same time. Beyond the issue of the dissociation between an implicit motor representation and more cognitive processing of spatial information, the issue of the interaction between these two systems is thus a matter of interest. It is suggested that the conscious, cognitive representation of a stimulus can contaminate or override the short-lived motor representation, but no reciprocal influence seem to occur. The interaction observed in patients can also be investigated in normals. The literature provides examples of interaction between sensorimotor and cognitive framing of space, which confirm that immediate action is not mediated by the same system as delayed action, and that elaborating a categorial representation of the action goal prevents the expression of the short-lived sensorimotor representation. It is concluded that action can be controlled by a sensory system which is specialized for on-line processing of relevant goal characteristics. The temporal constraints of this

  2. A multi-proxy approach to identifying short-lived marine incursions in the Early Carboniferous

    NASA Astrophysics Data System (ADS)

    Bennett, Carys; Davies, Sarah; Leng, Melanie; Snelling, Andrea; Millward, David; Kearsey, Timothy; Marshall, John; Reves, Emma

    2015-04-01

    This study is a contribution to the TW:eed Project (Tetrapod World: early evolution and diversification), which examines the rebuilding of Carboniferous ecosystems following a mass extinction at the end of the Devonian. The project focuses on the Tournaisian Ballagan Formation of Scotland and the Borders, which contains rare fish and tetrapod material. The Ballagan Formation is characterised by sandstones, dolomitic cementstones, paleosols, siltstones and gypsum deposits. The depositional environment ranges from fluvial, alluvial-plain to marginal-marine environments, with fluvial, floodplain and lacustrine deposition dominant. A multi-proxy approach combining sedimentology, palaeontology, micropalaeontology, palynology and geochemistry is used to identify short-lived marine transgressions onto the floodplain environment. Rare marginal marine fossils are: Chondrites-Phycosiphon, Spirorbis, Serpula, certain ostracod species, rare orthocones, brachiopods and putative marine sharks. More common non-marine fauna include Leiocopida and Podocopida ostracods, Mytilida and Myalinida bivalves, plants, eurypterids, gastropods and fish. Thin carbonate-bearing dolomitic cementstones and siltstone contain are the sedimentary deposits of marine incursions and occur throughout the formation. Over 600 bulk carbon isotope samples were taken from the 500 metre thick Norham Core (located near Berwick-Upon-Tweed), encompassing a time interval of around 13 million years. The results range from -26o to -19 δ13Corg, with an average of -19o much lighter than the average value for Early Carboniferous marine bulk organic matter (δ13C of -28 to -30). The isotope results correspond to broad-scale changes in the depositional setting, with more positive δ13C in pedogenic sediments and more negative δ13C in un-altered grey siltstones. They may also relate to cryptic (short-lived) marine incursions. A comparison of δ13C values from specific plant/wood fragments, palynology and bulk

  3. Separation efficiency of the MASHA facility for short-lived mercury isotopes

    NASA Astrophysics Data System (ADS)

    Rodin, A. M.; Belozerov, A. V.; Chernysheva, E. V.; Dmitriev, S. N.; Gulyaev, A. V.; Gulyaeva, A. V.; Itkis, M. G.; Kliman, J.; Kondratiev, N. A.; Krupa, L.; Novoselov, A. S.; Oganessian, Yu. Ts.; Podshibyakin, A. V.; Salamatin, V. S.; Siváček, I.; Stepantsov, S. V.; Vanin, D. V.; Vedeneev, V. Yu.; Yukhimchuk, S. A.; Granja, C.; Pospisil, S.

    2014-06-01

    The mass-separator MASHA built to identify Super Heavy Elements by their mass-to-charge ratios is described. The results of the off- and on-line measurements of its separation efficiency are presented. In the former case four calibrated leaks of noble gases were used. In the latter the efficiency was measured via 284 MeV Ar beam and with using the hot catcher. The ECR ion source was used in both cases. The -radioactive isotopes of mercury produced in the complete fusion reaction Ar+SmHg+xn were detected at the mass-separator focal plane. The half-lives and the separation efficiency for the short-lived mercury isotopes were measured. Potentialities of the MEDIPIX detector system have been demonstrated for future use at the mass-separator MASHA.

  4. Counteracting the climate effects of volcanic eruptions using short-lived greenhouse gases

    NASA Astrophysics Data System (ADS)

    Fuglestvedt, Jan S.; Samset, Bjørn H.; Shine, Keith P.

    2014-12-01

    A large volcanic eruption might constitute a climate emergency, significantly altering global temperature and precipitation for several years. Major future eruptions will occur, but their size or timing cannot be predicted. We show, for the first time, that it may be possible to counteract these climate effects through deliberate emissions of short-lived greenhouse gases, dampening the abrupt impact of an eruption. We estimate an emission pathway countering a hypothetical eruption 3 times the size of Mount Pinatubo in 1991. We use a global climate model to evaluate global and regional responses to the eruption, with and without counteremissions. We then raise practical, financial, and ethical questions related to such a strategy. Unlike the more commonly discussed geoengineering to mitigate warming from long-lived greenhouse gases, designed emissions to counter temporary cooling would not have the disadvantage of needing to be sustained over long periods. Nevertheless, implementation would still face significant challenges.

  5. The role of short-lived climate pollutants in meeting temperature goals

    NASA Astrophysics Data System (ADS)

    Bowerman, Niel H. A.; Frame, David J.; Huntingford, Chris; Lowe, Jason A.; Smith, Stephen M.; Allen, Myles R.

    2013-12-01

    Some recent high-profile publications have suggested that immediately reducing emissions of methane, black carbon and other short-lived climate pollutants (SLCPs) may contribute substantially towards the goal of limiting global warming to 2 °C above pre-industrial levels. Although this literature acknowledges that action on long-lived climate pollutants (LLCPs) such as CO2 is also required, it is not always appreciated that SLCP emissions in any given decade only have a significant impact on peak temperature under circumstances in which CO2 emissions are falling. Immediate action on SLCPs might potentially 'buy time' for adaptation by reducing near-term warming; however early SLCP reductions, compared with reductions in a future decade, do not buy time to delay reductions in CO2.

  6. The short-lived African turquoise killifish: an emerging experimental model for ageing.

    PubMed

    Kim, Yumi; Nam, Hong Gil; Valenzano, Dario Riccardo

    2016-02-01

    Human ageing is a fundamental biological process that leads to functional decay, increased risk for various diseases and, ultimately, death. Some of the basic biological mechanisms underlying human ageing are shared with other organisms; thus, animal models have been invaluable in providing key mechanistic and molecular insights into the common bases of biological ageing. In this Review, we briefly summarise the major applications of the most commonly used model organisms adopted in ageing research and highlight their relevance in understanding human ageing. We compare the strengths and limitations of different model organisms and discuss in detail an emerging ageing model, the short-lived African turquoise killifish. We review the recent progress made in using the turquoise killifish to study the biology of ageing and discuss potential future applications of this promising animal model. PMID:26839399

  7. The short-lived African turquoise killifish: an emerging experimental model for ageing

    PubMed Central

    Kim, Yumi; Nam, Hong Gil; Valenzano, Dario Riccardo

    2016-01-01

    ABSTRACT Human ageing is a fundamental biological process that leads to functional decay, increased risk for various diseases and, ultimately, death. Some of the basic biological mechanisms underlying human ageing are shared with other organisms; thus, animal models have been invaluable in providing key mechanistic and molecular insights into the common bases of biological ageing. In this Review, we briefly summarise the major applications of the most commonly used model organisms adopted in ageing research and highlight their relevance in understanding human ageing. We compare the strengths and limitations of different model organisms and discuss in detail an emerging ageing model, the short-lived African turquoise killifish. We review the recent progress made in using the turquoise killifish to study the biology of ageing and discuss potential future applications of this promising animal model. PMID:26839399

  8. Inter-laboratory comparisons of short-lived gamma-emitting radionuclides in nuclear reactor water.

    PubMed

    Klemola, S K

    2008-01-01

    Inter-laboratory comparisons of gamma-emitting nuclides in nuclear power plant coolant water have been carried out in Finland since 1994. The reactor water samples are taken and prepared by one of the two nuclear power plants and delivered to the participants. Since all the participants get their sample within just a few hours it has been possible to analyse and compare results of nuclides with half-lives shorter than 1h. The total number of short-lived nuclides is 26. All the main nuclides are regularly identified and the activities have been obtained with reasonable accuracy throughout the years. The overall deviation of the results has decreased in 13 years. The effects of true coincidence summing and discrepancies in nuclear data have been identified as potential sources of remaining discrepancies. All the participants have found this type of comparison very useful. PMID:18378157

  9. Short-lived radioisotopes scaling with energy in plasma focus device

    NASA Astrophysics Data System (ADS)

    Kakavandi, Javad A.; Roshan, Mahmood V.; Habibi, Morteza

    2016-03-01

    The computational investigation of the correlation between the achievable reaction yield and discharge energy for a plasma focus device (PFD) is presented. Radioisotope production in PFDs with applicable activities is highly dependent on establishing the related scaling law. Carbon target is bombarded by high energy deuterons and short-lived radioisotope of 13N is produced through 12C(d,n)13N in which the threshold energy is not very high. Both computed and measured ion energy spectra are used to estimate and optimize the scaling law. It is shown that the number of ions emitted from the pinch region for a device operating under optimized conditions is linearly proportional to the discharge energy of the PFD.

  10. Nanoelectrochemical approach to detecting short-lived intermediates of electrocatalytic oxygen reduction.

    PubMed

    Zhou, Min; Yu, Yun; Hu, Keke; Mirkin, Michael V

    2015-05-27

    Development of better catalysts for the oxygen reduction reaction (ORR) and other electrocatalytic processes requires detailed knowledge of reaction pathways and intermediate species. Here we report a new methodology for detecting charged reactive intermediates and its application to the mechanistic analysis of ORR. A nanopipette filled with an organic phase that is immiscible with the external aqueous solution was used as a tip in the scanning electrochemical microscope to detect and identify a short-lived superoxide (O2(●-)) intermediate and to determine the rate of its generation at the catalytic Pt substrate and its lifetime in neutral aqueous solution. The voltammogram of the O2(●-) anion transfer to the organic phase provides a unique signature for unambiguous identification of superoxide. The extremely short attainable separation distance between the pipette tip and substrate surface (∼1 nm) makes this technique suitable for detecting and identifying charged intermediates of catalytic processes with a lifetime of a few nanoseconds. PMID:25978070

  11. Laser spectroscopy of trapped short-lived Ra{sup +} ions

    SciTech Connect

    Versolato, O. O.; Giri, G. S.; Wansbeek, L. W.; Berg, J. E. van den; Hoek, D. J. van der; Jungmann, K.; Kruithof, W. L.; Onderwater, C. J. G.; Sahoo, B. K.; Santra, B.; Shidling, P. D.; Timmermans, R. G. E.; Willmann, L.; Wilschut, H. W.

    2010-07-15

    As an important step toward an atomic parity violation experiment in one single trapped Ra{sup +} ion, laser spectroscopy on short-lived {sup 212,213,214}Ra{sup +} ions was conducted. The isotope shift of the 6 {sup 2}D{sub 3/2}-7 {sup 2}P{sub 1/2} and 6 {sup 2}D{sub 3/2}-7 {sup 2}P{sub 3/2} transitions and the hyperfine structure constants of the 7 {sup 2}P{sub 1/2} and 6 {sup 2}D{sub 3/2} states in {sup 213}Ra{sup +} were measured, which provides a benchmark for the required atomic theory. A lower limit of 232(4) ms for 6 {sup 2}D{sub 5/2} state lifetime was determined.

  12. Short-lived oxygen diffusion during hot, deep-seated meteoric alteration of anorthosite

    PubMed

    Mora; Riciputi; Cole

    1999-12-17

    Heterogeneous oxygen isotope compositions of plagioclase from the Boehls Butte anorthosite include some of the most oxygen-18-depleted values (to -16 per mil) reported for plagioclase in meta-igneous rocks and indicate high-temperature (T > 500 degrees C) isotopic exchange between plagioclase and nearly pristine meteoric fluid. Retrograde reaction-enhanced permeability assisted influx of meteoric-hydrothermal fluids into the deep-seated anorthosite. Isotopic gradients of about 14 per mil over 600 micrometers in single crystals require short-lived (about 10(4) years) diffusional exchange of oxygen and locally large effective water:rock ratios, followed by rapid loss of water and cessation of oxygen diffusion in the anorthosite. PMID:10600738

  13. Seeds of alpine plants are short lived: implications for long-term conservation

    PubMed Central

    Mondoni, Andrea; Probert, Robin J.; Rossi, Graziano; Vegini, Emanuele; Hay, Fiona R.

    2011-01-01

    Background and Aims Alpine plants are considered one of the groups of species most sensitive to the direct and indirect threats to ecosystems caused by land use and climate change. Collecting and banking seeds of plant species is recognized as an effective tool for providing propagating material to re-establish wild plant populations and for habitat repair. However, seeds from cold wet environments have been shown to be relatively short lived in storage, and therefore successful long-term seed conservation for alpine plants may be difficult. Here, the life spans of 69 seed lots representing 63 related species from alpine and lowland locations from northern Italy are compared. Methods Seeds were placed into experimental storage at 45 °C and 60 % relative humidity (RH) and regularly sampled for germination. The time taken in storage for viability to fall to 50 % (p50) was determined using probit analysis and used as a measure of relative seed longevity between seed lots. Key Results Across species, p50 at 45 °C and 60 % RH varied from 4·7 to 95·5 d. Seed lots from alpine populations/species had significantly lower p50 values compared with those from lowland populations/species; the lowland seed lots showed a slower rate of loss of germinability, higher initial seed viability, or both. Seeds were progressively longer lived with increased temperature and decreased rainfall at the collecting site. Conclusions Seeds of alpine plants are short lived in storage compared with those from lowland populations/related taxa. The lower resistance to ageing in seeds of alpine plants may arise from low selection pressure for seed resistance to ageing and/or damage incurred during seed development due to the cool wet conditions of the alpine climate. Long-term seed conservation of several alpine species using conventional seed banking methods will be problematic. PMID:21081585

  14. Global Air Quality and Climate Impacts of Mitigating Short-lived Climate Pollution in China

    NASA Astrophysics Data System (ADS)

    Harper, K.; Unger, N.; Heyes, C.; Kiesewetter, G.; Klimont, Z.; Schoepp, W.; Wagner, F.

    2014-12-01

    China is a major emitter of harmful air pollutants, including the short-lived climate pollutants (SLCPs) and their precursors. Implementation of pollution control technologies provides a mechanism for simultaneously protecting human and ecosystem health and achieving near-term climate co-benefits; however, predicting the outcomes of technical and policy interventions is challenging because the SLCPs participate in both climate warming and cooling and share many common emission sources. Here, we present the results of a combined regional integrated assessment and global climate modeling study aimed at quantifying the near-term climate and air quality co-benefits of selective control of Chinese air pollution emissions. Results from IIASA's Greenhouse Gas - Air Pollution Interactions and Synergies (GAINS) integrated assessment model indicate that methane emission reductions make up > 75% of possible CO2-equivalent emission reductions of the SLCPs and their precursors in China in 2030. A multi-pollutant emission reduction scenario incorporating the 2030 Chinese pollution control measures with the highest potential for future climate impact is applied to the NASA ModelE2 - Yale Interactive Terrestrial Biosphere (NASA ModelE2-YIBs) global carbon - chemistry - climate model to assess the regional and long-range impacts of Chinese SLCP mitigation measures. Using model simulations that incorporate dynamic methane emissions and photosynthesis-dependent isoprene emissions, we quantify the impacts of Chinese reductions of the short-lived air pollutants on radiative forcing and on surface ozone and particulate air pollution. Present-day modeled methane mole fractions are evaluated against SCIAMACHY methane columns and NOAA ESRL/GMD surface flask measurements.

  15. Muscle senescence in short-lived wild mammals, the soricine shrews Blarina brevicauda and Sorex palustris.

    PubMed

    Hindle, Allyson G; Lawler, John M; Campbell, Kevin L; Horning, Markus

    2009-06-01

    Red-toothed (soricine) shrews are consummate predators exhibiting the highest energy turnovers and shortest life spans (ca. 18 months) of any mammal, yet virtually nothing is known regarding their physiological aging. We assessed the emerging pattern of skeletal muscle senescence (contractile/connective tissue components) in sympatric species, the semi-aquatic water shrew (WS), Sorex palustris, and the terrestrial short-tailed shrew (STS), Blarina brevicauda, to determine if muscle aging occurs in wild, short-lived mammals (H(0): shrews do not survive to an age where senescence occurs), and if so, whether these alterations are species-specific. Gracilis muscles were collected from first-year (n=17) and second-year (n=17) field-caught shrews. Consistent with typical mammalian aging, collagen content (% area) increased with age in both species (S. palustris: approximately 50%; B. brevicauda: approximately 60%). Muscle was dominated by stiffer Type I collagen, and the ratio of collagen Type I:Type III more than doubled with age. The area ratio of muscle:collagen decreased with age in both species, but was considerably lower in adult STS, suggesting species-specificity of senescence. Extracellular space was age-elevated in B. brevicauda, but was preserved in S. palustris ( approximately 50 vs. 10% elevation). Though juvenile interspecific comparisons revealed no significance, adult WS myocytes had 68% larger cross-sectional area and occurred at 28% lower fibers/area than those of adult STS. We demonstrate that age-related muscle senescence does occur in wild-caught, short-lived mammals, and we therefore reject this classic aging theory tenet. Our findings moreover illustrate that differential age adjustments in contractile/connective tissue components of muscle occur in the two species of wild-caught shrews. PMID:19296507

  16. Power-density spectrum of non-stationary short-lived light curves

    NASA Astrophysics Data System (ADS)

    Guidorzi, Cristiano

    2011-08-01

    The power-density spectrum of a light curve is often calculated as the average of a number of spectra derived on individual time intervals the light curve is divided into. This procedure implicitly assumes that each time interval is a different sample function of the same stochastic ergodic process. While this assumption can be applied to many astrophysical sources, there remains a class of transient, highly non-stationary and short-lived events, such as gamma-ray bursts, for which this approach is often inadequate. The power spectrum statistics of a constant signal affected by statistical (Poisson) noise are known to be a χ22 in the Leahy normalization. However, this is no more the case when a non-stationary signal is also present. As a consequence, the uncertainties on the power spectrum cannot be calculated on the basis of the χ22 properties, as assumed by tools such as XRONOS POWSPEC. We generalize the result in the case of a non-stationary signal affected by uncorrelated white noise and show that the new distribution is a non-central χ22(λ), whose non-central value λ is the power spectrum of the deterministic function describing the non-stationary signal. Finally, we test these results in the case of synthetic curves of gamma-ray bursts. We end up with a new formula for calculating the power spectrum uncertainties. This is crucial in the case of non-stationary short-lived processes affected by uncorrelated statistical noise, for which ensemble averaging does not make any physical sense.

  17. CARIBIC observations of short-lived halocarbons and carbonyl sulphide over Asia

    NASA Astrophysics Data System (ADS)

    Leedham, E.; Wisher, A.; Oram, D.; Baker, A. K.; Brenninkmeijer, C. A.

    2013-12-01

    The CARIBIC project (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container, www.caribic-atmospheric.com) aims to investigate the spatial and temporal distribution of a wide-range of compounds, including those of marine origin/influence, via ~monthly flights to collect in situ data and whole air samples aboard a commercial Lufthansa aircraft. CARIBIC measures up to an altitude of 12 km, allowing the influence of marine compounds on the upper troposphere/lower stratosphere (UTLS) to be explored. In particular, CARIBIC is a useful tool for exploring the impact of very short lived halocarbons (e.g. CH2Br2, CHBr3), whose impact on stratospheric ozone is dependent on convective uplift to the UTLS, a process which is not yet fully quantified. As part of the suite of CARIBIC measurements, whole air samples are analysed at the University of East Anglia (UEA) via gas chromatography mass spectrometry for carbonyl sulphide (OCS) and up to 40 halocarbons (accounting for virtually 100% of organic chlorine, bromine and iodine in the UTLS). Here we present an overview of short-lived halocarbons and OCS measured by CARIBIC. We focus on two regions of particular interest. (1) measurements made in 2012 over the tropical west Pacific to link with UEA measurements made during the SHIVA campaign. (2) measurements made during a collection of flights over India in 2008. Flights over India investigated the impact of monsoon circulation on the distribution of these compounds; for example, elevated concentrations of OCS were seen in CARIBIC samples taken over India during the summer monsoon (July - September). These flights, along with a wider range of flights over Asia (from Frankfurt to Guangzhou, Manila, Bangkok and Kuala Lumpur) can provide unique information on the influence of tropical convection and monsoon circulation on halocarbon and OCS transport within this region.

  18. Long- and short-lived nuclide constraints on the recent evolution of permafrost soils

    NASA Astrophysics Data System (ADS)

    Bagard, M.; Chabaux, F. J.; Rihs, S.; Pokrovsky, O. S.; Prokushkin, A. S.; Viers, J.

    2011-12-01

    Frozen permafrost ecosystems are particularly sensitive to climate warming, which notably induces a deepening of the active layer (the maximum thawing depth during summer time). As a consequence, geochemical and hydrological fluxes within boreal areas are expected to be significantly affected in the future. Understanding the relationship between environmental changes and permafrost modifications is then a major challenge. This work aims to evaluate in a Siberian watershed the dynamics of the permafrost active layer and their recent modifications by combining a classic study of long-lived nuclides to the study of short-lived nuclides of U and Th decay series. Two soil profiles, located on opposite slopes (north- and south-facing slopes) of the Kulingdakan watershed (Putorana Plateau, Central Siberia), were sampled at several depths within the active layer and (238U), (234U), (232Th), (230Th), (226Ra), (228Ra), (228Th) and (210Pb) were measured on bulk soil samples by TIMS or gamma spectrometry. Our results show that south-facing and north-facing soil profiles are significantly different in terms of evolution of chemical concentrations and nuclide activities; north-facing soil profile is strongly affected by atmospheric inputs whereas long-lived nuclide dynamics within south-facing soil profile are dominated by weathering and exhibit more complex patterns. The amount of above-ground biomass being the single varying parameter between the two slopes of the watershed, we suggest that the structuring of permafrost active layer is very sensitive to vegetation activity and that the functioning of boreal soils will be significantly modified by its development due to more favorable climatic conditions. Moreover, the coupling of long and short-lived nuclides highlights the superimposition of a recent mobilization of chemical elements within soils (<10 years) over a much older soil structure (>8000 years), which can be observed for both soil profiles. The shallowest layer of

  19. The impacts of short-lived ozone precursors on climate and air quality

    NASA Astrophysics Data System (ADS)

    Fry, Meridith McGee

    Human emissions of short-lived ozone precursors not only degrade air quality and health, but indirectly affect climate via chemical effects on ozone, methane, and aerosols. Some have advocated for short-lived air pollutants in near-term climate mitigation strategies, in addition to national air quality programs, but their radiative forcing (RF) impacts are uncertain and vary based on emission location. In this work, global chemical transport modeling is combined with radiative transfer modeling to study the impacts of regional ozone precursor emissions (NOx, CO, and NMVOCs) on climate, via changes in ozone, methane, and sulfate, and on regional and global air quality. The first study evaluates NOx, CO, and NMVOC emission reductions from four regions across an ensemble of models, finding that NMVOC and CO reductions from all four regions cool climate (negative RF) by decreasing ozone and methane, while improving air quality. NOx and NMVOC global warming potentials (GWPs), a measure of the relative radiative effects of individual climate forcers, vary strongly among regions, while CO GWPs show less variability. The second and third studies investigate further the RF and air quality impacts of CO and NMVOC emission reductions from 10 world regions. The greatest benefits to RF and air quality (per unit emissions) are achieved by CO reductions from the tropics, due to more active photochemistry and convection. CO GWPs are fairly independent of the reduction region (GWP20: 3.71 to 4.37; GWP100: 1.26 to 1.44), while NMVOC GWPs are more variable (GWP 20: -1.13 to 18.9; GWP100: 0.079 to 6.05). Accounting for additional forcings from CO and NMVOC emissions would likely change RF and GWP estimates. Regionally-specific GWPs for NOx and NMVOCs and a globally-uniform GWP for CO may allow these gases to be included in a multi-gas emissions trading framework, and enable comprehensive strategies for meeting climate and air quality goals simultaneously. Future research could

  20. Counteracting the climate effects of volcanic eruptions using short-lived greenhouse gases

    NASA Astrophysics Data System (ADS)

    Samset, B. H.; Fuglestvedt, J.; Shine, K. P.

    2014-12-01

    A large volcanic eruption might constitute a climate emergency, significantly altering global temperature and precipitation for several years. Major future eruptions will occur, but their size or timing cannot be predicted. How could global society prepare for, and react to, such emergencies? One possibility is deliberate, coordinated emissions of short-lived greenhouse gases, along a pathway designed to match the climate responses to the eruption. We estimate such an emission pathway, countering a hypothetical eruption three times the size of Mt Pinatubo in 1991. Using a global climate model to evaluate global and regional responses to the eruption, with and without counter emissions, we show that it may be possible to counteract its climate effects, significantly dampening the abrupt impact of the eruption. We then raise practical, financial and ethical aspects related to such a strategy. Designed emissions to counter temporary global cooling would not have the disadvantages associated with more commonly discussed geoengineering to avoid long-term warming. Nevertheless, implementation would still face significant challenges.

  1. A platform for rapid exploration of aging and diseases in a naturally short-lived vertebrate

    PubMed Central

    Harel, Itamar; Benayoun, Bérénice A.; Machado, Ben; Singh, Param Priya; Hu, Chi-Kuo; Pech, Matthew F.; Valenzano, Dario R.; Zhang, Elisa; Sharp, Sabrina C.; Artandi, Steven E.; Brunet, Anne

    2015-01-01

    Summary Aging is a complex process that affects multiple organs. Modeling aging and age-related diseases in the lab is challenging because classical vertebrate models have relatively long lifespans. Here we develop the first platform for rapid exploration of age-dependent traits and diseases in vertebrates, using the naturally short-lived African turquoise killifish. We provide an integrative genomic and genome-editing toolkit in this organism using our de novo-assembled genome and the CRISPR/Cas9 technology. We mutate many genes encompassing the hallmarks of aging, and for a subset, we produce stable lines within 2–3 months. As a proof-of-principle, we show that fish deficient for the protein subunit of telomerase exhibit the fastest onset of telomere-related pathologies among vertebrates. We further demonstrate the feasibility of creating specific genetic variants. This genome-to-phenotype platform represents a unique resource for studying vertebrate aging and disease in a high throughput manner and for investigating candidates arising from human genome-wide studies. PMID:25684364

  2. Mitigation of short-lived climate pollutants slows sea-level rise

    NASA Astrophysics Data System (ADS)

    Hu, Aixue; Xu, Yangyang; Tebaldi, Claudia; Washington, Warren M.; Ramanathan, Veerabhadran

    2013-08-01

    Under present growth rates of greenhouse gas and black carbon aerosol emissions, global mean temperatures can warm by as much as 2°C from pre-industrial temperatures by about 2050. Mitigation of the four short-lived climate pollutants (SLCPs), methane, tropospheric ozone, hydrofluorocarbons and black carbon, has been shown to reduce the warming trend by about 50% (refs , ) by 2050. Here we focus on the potential impact of this SLCP mitigation on global sea-level rise (SLR). The temperature projections under various SLCP scenarios simulated by an energy-balance climate model are integrated with a semi-empirical SLR model, derived from past trends in temperatures and SLR, to simulate future trends in SLR. A coupled ocean-atmosphere climate model is also used to estimate SLR trends due to just the ocean thermal expansion. Our results show that SLCP mitigation can have significant effects on SLR. It can decrease the SLR rate by 24-50% and reduce the cumulative SLR by 22-42% by 2100. If the SLCP mitigation is delayed by 25 years, the warming from pre-industrial temperature exceeds 2°C by 2050 and the impact of mitigation actions on SLR is reduced by about a third.

  3. Growth in stratospheric chlorine from short-lived chemicals not controlled by the Montreal Protocol

    NASA Astrophysics Data System (ADS)

    Hossaini, R.; Chipperfield, M. P.; Saiz-Lopez, A.; Harrison, J. J.; Glasow, R.; Sommariva, R.; Atlas, E.; Navarro, M.; Montzka, S. A.; Feng, W.; Dhomse, S.; Harth, C.; Mühle, J.; Lunder, C.; O'Doherty, S.; Young, D.; Reimann, S.; Vollmer, M. K.; Krummel, P. B.; Bernath, P. F.

    2015-06-01

    We have developed a chemical mechanism describing the tropospheric degradation of chlorine containing very short-lived substances (VSLS). The scheme was included in a global atmospheric model and used to quantify the stratospheric injection of chlorine from anthropogenic VSLS ( ClyVSLS) between 2005 and 2013. By constraining the model with surface measurements of chloroform (CHCl3), dichloromethane (CH2Cl2), tetrachloroethene (C2Cl4), trichloroethene (C2HCl3), and 1,2-dichloroethane (CH2ClCH2Cl), we infer a 2013 ClyVSLS mixing ratio of 123 parts per trillion (ppt). Stratospheric injection of source gases dominates this supply, accounting for ˜83% of the total. The remainder comes from VSLS-derived organic products, phosgene (COCl2, 7%) and formyl chloride (CHClO, 2%), and also hydrogen chloride (HCl, 8%). Stratospheric ClyVSLS increased by ˜52% between 2005 and 2013, with a mean growth rate of 3.7 ppt Cl/yr. This increase is due to recent and ongoing growth in anthropogenic CH2Cl2—the most abundant chlorinated VSLS not controlled by the Montreal Protocol.

  4. Dissolved organic matter composition drives the marine production of brominated very short-lived substances.

    PubMed

    Liu, Yina; Thornton, Daniel C O; Bianchi, Thomas S; Arnold, William A; Shields, Michael R; Chen, Jie; Yvon-Lewis, Shari A

    2015-03-17

    Brominated very short-lived substances (BrVSLS), such as bromoform, are important trace gases for stratospheric ozone chemistry. These naturally derived trace gases are formed via bromoperoxidase-mediated halogenation of dissolved organic matter (DOM) in seawater. Information on DOM type in relation to the observed BrVSLS concentrations in seawater, however, is scarce. We examined the sensitivity of BrVSLS production in relation to the presence of specific DOM moieties. A total of 28 model DOM compounds in artificial seawater were treated with vanadium bromoperoxidase (V-BrPO). Our results show a clear dependence of BrVSLS production on DOM type. In general, molecules that comprise a large fraction of the bulk DOM pool did not noticeably affect BrVSLS production. Only specific cell metabolites and humic acid appeared to significantly enhance BrVSLS production. Amino acids and lignin phenols suppressed enzyme-mediated BrVSLS production and may instead have formed halogenated nonvolatile molecules. Dibromomethane production was not observed in any experiments, suggesting it is not produced by the same pathway as the other BrVSLS. Our results suggest that regional differences in DOM composition may explain the observed BrVSLS concentration variability in the global ocean. Ultimately, BrVSLS production and concentrations are likely affected by DOM composition, reactivity, and cycling in the ocean. PMID:25723123

  5. Multi-model evaluation of short-lived pollutant distributions over East Asia during summer 2008

    NASA Astrophysics Data System (ADS)

    Quennehen, B.; Raut, J.-C.; Law, K. S.; Ancellet, G.; Clerbaux, C.; Kim, S.-W.; Lund, M. T.; Myhre, G.; Olivié, D. J. L.; Safieddine, S.; Skeie, R. B.; Thomas, J. L.; Tsyro, S.; Bazureau, A.; Bellouin, N.; Daskalakis, N.; Hu, M.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Myriokefalitakis, S.; Quaas, J.; Rumbold, S. T.; Schulz, M.; Cherian, R.; Shimizu, A.; Wang, J.; Yoon, S.-C.; Zhu, T.

    2015-04-01

    The ability of six global and one regional model to reproduce distributions of tropospheric ozone and its precursors, as well as aerosols over Asia in summer 2008 is evaluated using satellite and in-situ observations. Whilst ozone precursors (NO2 and CO) are generally underestimated by the models in the troposphere, surface NO2 concentrations are overestimated, suggesting that emissions of NOx are too high. Ozone integrated columns and vertical profiles are generally well modeled, but the global models face difficulties simulating the ozone gradient at the surface between urban and rural environments, pointing to the need to increase model resolution. The accuracy of simulated aerosol patterns over eastern China and northern India varies between the models, and although most of the models reproduce the observed pollution features over eastern China, significant biases are noted in the magnitude of optical properties (aerosol optical depth, aerosol backscatter). These results have important implications for accurate prediction of pollution episodes affecting air quality and the radiative effects of these short-lived climate pollutants over Asia.

  6. Early auxin-induced genes encode short-lived nuclear proteins.

    PubMed Central

    Abel, S; Oeller, P W; Theologis, A

    1994-01-01

    The plant growth hormone indoleacetic acid (IAA) transcriptionally activates gene expression in plants. Some of the genes whose expression is induced by IAA encode a family of proteins in pea (PS-IAA4 and PS-IAA6) and Arabidopsis (IAA1 and IAA2) that contain putative nuclear localization signals that direct a beta-glucuronidase reporter protein into the nucleus. Pulse-chase and immunoprecipitation experiments have defined the t1/2 of the PS-IAA4 and PS-IAA6 proteins to be 8 and 6 min, respectively. Their most prominent feature is the presence of a beta alpha alpha motif similar to the beta-sheet DNA-binding domain found in prokaryotic repressors of the Arc family. Based on these data, we suggest that plant tissues express short-lived nuclear proteins as a primary response to IAA. We propose that these proteins act as activators or repressors of genes responsible for mediating the various auxin responses. Images Fig. 2 Fig. 3 Fig. 4 PMID:8278386

  7. A new approach for fluid dynamics simulation: The Short-lived Water Cuboid Particle model

    NASA Astrophysics Data System (ADS)

    Qiao, Changjian; Li, Jiansong; Tian, Zongshun

    2016-09-01

    There are many researches to simulate the fluid which adopt the traditional particle-based approach and the grid-based approach. However, it needs massive storage in the traditional particle-based approach and it is very complicated to design the grid-based approach with the Navier-Stokes Equations or the Shallow Water Equations (SWEs) because of the difficulty of solving equations. This paper presents a new model called the Short-lived Water Cuboid Particle model. It updates the fluid properties (mass and momentum) recorded in the fixed Cartesian grids by computing the weighted sum of the water cuboid particles with a time step life. Thus it is a two-type-based approach essentially, which not only owns efficient computation and manageable memory like the grid-based approach, but also deals with the discontinuous water surface (wet/dry fronts, boundary conditions, etc.) with high accuracy as well as the particle-based approach. The proposed model has been found capable to simulate the fluid excellently for three laboratory experimental cases and for the field case study of the Malpasset dam-break event occurred in France in 1959. The obtained results show that the model is proved to be an alternative approach to simulate the fluid dynamics with a fair accuracy.

  8. Integrated measurements of short-lived 222Rn progeny by rotating filters.

    PubMed

    Pressyanov, D S; Guelev, M G; Pentchev, O J

    1993-05-01

    The dependence of the risk from inhalation of radon progeny on their disequilibrium suggests that the measurements of the time-integrated concentrations of each of the short-lived radon progeny are necessary for complete risk estimations. This paper presents a method that, in principle, allows the determination of the integrated specific volume activities in air of each of the radionuclides 218Po, 214Pb, 214Bi, 212Pb, and 212Bi. The method employs thermoluminescence detectors positioned around uniformly rotating filters. Two prototypes that are suitable for practical applications are described and mathematical expressions for data processing are given. Experiments with these "rotating filter dosimeters" were conducted in atmospheres radiologically dominated by 222Rn progeny. The comparison between the results obtained by the proposed method and those given by simultaneously conducted series of instantaneous grab-sampling measurements support the conclusion that the method works for 222Rn progeny. The method can be experimentally extended for 220Rn progeny as well as for unattached fractions. PMID:8387983

  9. Age-dependent decline in fin regenerative capacity in the short-lived fish Nothobranchius furzeri

    PubMed Central

    Wendler, Sebastian; Hartmann, Nils; Hoppe, Beate; Englert, Christoph

    2015-01-01

    The potential to regenerate declines with age in a wide range of organisms. A popular model system to study the mechanisms of regeneration is the fin of teleost fish, which has the ability to fully regrow upon amputation. Here, we used the short-lived killifish Nothobranchius furzeri to analyse the impact of aging on fin regeneration in more detail. We observed that young fish were able to nearly completely (98%) regenerate their amputated caudal fins within 4 weeks, whereas middle-aged fish reached 78%, old fish 57% and very old fish 46% of their original fin size. The difference in growth rate between young and old fish was already significant at 3 days post amputation (dpa) and increased with time. We therefore hypothesized that early events are crucial for the age-related differences in regenerative capacity. Indeed, we could observe a higher percentage of proliferating cells in early regenerating fin tissue of young fish compared with aged fish and larger fractions of apoptotic cells in aged fish. Furthermore, young fish showed peak upregulation of several genes involved in fgf and wnt/β-catenin signalling at an earlier time point than old fish. Our findings suggest that regenerative processes are initiated earlier and that regeneration overall is more efficient in younger fish. PMID:26121607

  10. Harvard-MIT research program in short-lived radiopharmaceuticals. Final report

    SciTech Connect

    Adelstein, S.J.

    1995-02-01

    The Harvard-MIT Research Program in Short-lived Radiopharmaceuticals was established in 1977 to foster interaction among groups working in radiopharmaceutical chemistry at Harvard Medical School, the Massachusetts Institute of Technology, and the Massachusetts General Hospital. To this was added a group at The Childrens Hospital. From these collaborations and building upon the special strengths of the participating individuals, laboratories and institutions, it was hoped that original approaches would be found for the design of new, clinically useful, radiolabeled compounds. The original thrust of this proposal included: (a) examination of the coordination chemistry of technetium as a basis for rational radiopharmaceutical design, (b) development of an ultrashort-lived radionuclide generator for the diagnosis of congenital heart disease in newborns, (c) synthesis of receptor-site-directed halopharmaceuticals, (d) improved facile labeling of complex molecules with positron-emitting radionuclides. The authors` 1986 proposal was oriented toward organs and disease, emphasizing radiolabeled agents that delineate specific functions and the distribution of receptors in brain, heart, and tumors. In 1989, they further refined their purposes and focused on two major aims: (a) synthesis and utilization of neutral technetium and rhenium complexes of high specific activity, and (b) development of new approaches to the radiolabeling of proteins, peptides, immunoglobulins, and their fragments. In 1992, the authors amended this proposal to concentrate their efforts on biologically active peptides and proteins for targeted radiodiagnosis and therapy.

  11. Recovery of short-lived chemical species in a couette flow reactor

    SciTech Connect

    Ouyang, Q.; Swinney, H.L. ); Roux, J.C.; Kepper, P.; Boissonade, J. )

    1992-04-01

    This paper reports on a new technique for studying and recovering short-lived chemical intermediate species that has been developed using a Couette reactor, which is an open one-dimensional reaction-diffusion system. Reaction occurs in the annulus between concentric cylinders with the inner one rotating and the outer one at rest. Fresh reagents are in contact with the ends of the annulus, but there is no net axial flow. The axial transport arising from the hydrodynamic motion is effectively diffusive, but has a diffusion coefficient 3 to 5 order of magnitude larger than that of molecular diffusion. The oxidant (ClO{sub 2}{sup {minus}}) and reductant (I{sup {minus}}) of an autocatalytic reaction are fed at opposite ends of the reactor. The reactants diffuse toward each other and react, forming a steady, sharp chemical front and a stable spatial concentration band of unstable intermediate species (HOCl) in the front region. Unstable intermediate species are thus stabilized at a well-defined spatial position where they can be recovered and studied. The experiments and numerical simulations demonstrate that the faster the reaction rate, the stabler the chemical front and the more effective the recovery of unstable intermediate species.

  12. New use of global warming potentials to compare cumulative and short-lived climate pollutants

    NASA Astrophysics Data System (ADS)

    Allen, Myles R.; Fuglestvedt, Jan S.; Shine, Keith P.; Reisinger, Andy; Pierrehumbert, Raymond T.; Forster, Piers M.

    2016-08-01

    Parties to the United Nations Framework Convention on Climate Change (UNFCCC) have requested guidance on common greenhouse gas metrics in accounting for Nationally determined contributions (NDCs) to emission reductions. Metric choice can affect the relative emphasis placed on reductions of `cumulative climate pollutants' such as carbon dioxide versus `short-lived climate pollutants' (SLCPs), including methane and black carbon. Here we show that the widely used 100-year global warming potential (GWP100) effectively measures the relative impact of both cumulative pollutants and SLCPs on realized warming 20-40 years after the time of emission. If the overall goal of climate policy is to limit peak warming, GWP100 therefore overstates the importance of current SLCP emissions unless stringent and immediate reductions of all climate pollutants result in temperatures nearing their peak soon after mid-century, which may be necessary to limit warming to ``well below 2 °C'' (ref. ). The GWP100 can be used to approximately equate a one-off pulse emission of a cumulative pollutant and an indefinitely sustained change in the rate of emission of an SLCP. The climate implications of traditional CO2-equivalent targets are ambiguous unless contributions from cumulative pollutants and SLCPs are specified separately.

  13. Short-Lived Buildings in China: Impacts on Water, Energy, and Carbon Emissions.

    PubMed

    Cai, Wenjia; Wan, Liyang; Jiang, Yongkai; Wang, Can; Lin, Lishen

    2015-12-15

    This paper has changed the vague understanding that "the short-lived buildings have huge environmental footprints (EF)" into a concrete one. By estimating the annual floor space of buildings demolished and calibrating the average building lifetime in China, this paper compared the EF under various assumptive extended buildings' lifetime scenarios based on time-series environmental-extended input-output model. Results show that if the average buildings' lifetime in China can be extended from the current 23.2 years to their designed life expectancy, 50 years, in 2011, China can reduce 5.8 Gt of water withdrawal, 127.1 Mtce of energy consumption, and 426.0 Mt of carbon emissions, each of which is equivalent to the corresponding annual EF of Belgium, Mexico, and Italy. These findings will urge China to extend the lifetime of existing and new buildings, in order to reduce the EF from further urbanization. This paper also verifies that the lifetime of a product or the replacement rate of a sector is a very important factor that influences the cumulative EF. When making policies to reduce the EF, adjusting people's behaviors to extend the lifetime of products or reduce the replacement rate of sectors may be a very simple and cost-effective option. PMID:26561867

  14. Simulating the impact of emissions of brominated very short lived substances on past stratospheric ozone trends

    NASA Astrophysics Data System (ADS)

    Sinnhuber, Björn-Martin; Meul, Stefanie

    2015-04-01

    Bromine from very short lived substances (VSLS), primarily from natural oceanic sources, contributes substantially to the stratospheric bromine loading. This source of stratospheric bromine has so far been ignored in most chemistry climate model calculations of stratospheric ozone trends. Here we present a transient simulation with the chemistry climate model EMAC for the period 1960-2005 including emissions of the five brominated VSLS CHBr3, CH2Br2, CH2BrCl, CHBrCl2, and CHBr2Cl. The emissions lead to a realistic stratospheric bromine loading of about 20 pptv for present-day conditions. Comparison with a standard model simulation without VSLS shows large differences in modeled ozone in the extratropical lowermost stratosphere and in the troposphere. Differences in ozone maximize in the Antarctic Ozone Hole, resulting in more than 20% less ozone when VSLS are included. Even though the emissions of VSLS are assumed to be constant in time, the model simulation with VSLS included shows a much larger ozone decrease in the lowermost stratosphere during the 1979-1995 period and a faster ozone increase during 1996-2005, in better agreement with observed ozone trends than the standard simulation without VSLS emissions.

  15. Light-ion-induced reactions in mass measurements of neutron-deficient nuclides close to A = 100

    NASA Astrophysics Data System (ADS)

    Elomaa, V.-V.; Eronen, T.; Hager, U.; Hakala, J.; Jokinen, A.; Kankainen, A.; Moore, I. D.; Rahaman, S.; Rissanen, J.; Rubchenya, V.; Weber, C.; Äystö, J.

    2009-04-01

    A survey of neutron-deficient nuclides which can be produced via proton- and 3He -induced fusion-evaporation reactions in the A = 100 region was made using a Penning trap as a high-resolution mass filter. A comparison of the measured isotopic rates with a statistical model calculation for the proton-induced reactions shows the importance of using the precise binding energy values for the final reaction products. In particular, proton separation energies were found to play an important role in the evaporation process. In addition, accurate masses of 12 nuclides, 97-99, 101Pd , 100Ag , 101-105Cd and 102, 104In , were determined with uncertainties of less than 10keV.

  16. Mass Measurements of Very Neutron-Deficient Mo and Tc Isotopes and Their Impact on rp Process Nucleosynthesis

    SciTech Connect

    Haettner, E.; Plass, W. R.; Scheidenberger, C.; Ackermann, D.; Block, M.; Eliseev, S.; Herfurth, F.; Hessberger, F. P.; Hofmann, S.; Kluge, H.-J.; Audi, G.; Blaum, K.; Ketter, J.; Fleckenstein, T.; Ketelaer, J.; Marx, G.; Schweikhard, L.; Mazzocco, M.; Novikov, Yu. N.; Vorobjev, G.

    2011-03-25

    The masses of ten proton-rich nuclides, including the N=Z+1 nuclides {sup 85}Mo and {sup 87}Tc, were measured with the Penning trap mass spectrometer SHIPTRAP. Compared to the Atomic Mass Evaluation 2003 a systematic shift of the mass surface by up to 1.6 MeV is observed causing significant abundance changes of the ashes of astrophysical x-ray bursts. Surprisingly low {alpha} separation energies for neutron-deficient Mo and Tc are found, making the formation of a ZrNb cycle in the rp process possible. Such a cycle would impose an upper temperature limit for the synthesis of elements beyond Nb in the rp process.

  17. Comment on ``Existence of long-lived isomeric states in naturally-occurring neutron-deficient Th isotopes''

    NASA Astrophysics Data System (ADS)

    Barber, R. C.; de Laeter, J. R.

    2009-04-01

    In their article “Existence of Long-Lived Isomeric States in Naturally-Occuring Neutron-Deficient Th Isotopes” [Phys. Rev. C 76, 021303 (2007)], Marinov fail to demonstrate that basic mass spectrometric protocols, such as abundance sensitivity, linearity, and freedom from possible interferences, have been met. In particular, the claim that four isomeric states of Th have been discovered, using an inductively coupled plasma-sector field mass spectrometer (ICP-SFMS), with abundances from (1-10)×10-11 relative to Th232, cannot be accepted, given the known abundance sensitivities of other sector field mass spectrometers. Accelerator mass spectrometry is the only mass spectrometric methodology capable of measuring relative abundances of the magnitude claimed by Marinov

  18. Mass measurements of very neutron-deficient Mo and Tc isotopes and their impact on rp process nucleosynthesis.

    PubMed

    Haettner, E; Ackermann, D; Audi, G; Blaum, K; Block, M; Eliseev, S; Fleckenstein, T; Herfurth, F; Hessberger, F P; Hofmann, S; Ketelaer, J; Ketter, J; Kluge, H-J; Marx, G; Mazzocco, M; Novikov, Yu N; Plass, W R; Rahaman, S; Rauscher, T; Rodríguez, D; Schatz, H; Scheidenberger, C; Schweikhard, L; Sun, B; Thirolf, P G; Vorobjev, G; Wang, M; Weber, C

    2011-03-25

    The masses of ten proton-rich nuclides, including the N=Z+1 nuclides ⁸⁵Mo and ⁸⁷Tc, were measured with the Penning trap mass spectrometer SHIPTRAP. Compared to the Atomic Mass Evaluation 2003 a systematic shift of the mass surface by up to 1.6 MeV is observed causing significant abundance changes of the ashes of astrophysical x-ray bursts. Surprisingly low α separation energies for neutron-deficient Mo and Tc are found, making the formation of a ZrNb cycle in the rp process possible. Such a cycle would impose an upper temperature limit for the synthesis of elements beyond Nb in the rp process. PMID:21517310

  19. Measurement of Short-Lived Fission-Product Yields of URANIUM-235 Using High-Resolution Gamma Spectra.

    NASA Astrophysics Data System (ADS)

    Tipnis, Sameer Vijay

    Independent yields of short-lived fission products produced by the thermal neutron induced fission of ^{235}U were determined from the measurements of high resolution gamma spectra. Comparisons were made to the recommended yield values tabulated in the ENDF/B-VI evaluated fission-product data base. Measurements of the gamma spectra were made with a high purity germanium detector (HPGe) using a NaI(Tl) annulus for Compton suppression. Use of beta-gamma coincidence reduced the random background and also allowed a precise definition of the delay time. The experiment was carried out at the 5.5 MV Van de Graaff facility at the University of Massachusetts Lowell. Rapid transfer of the fission fragments to a low background counting environment, a crucial factor in determining the yields of short-lived fission products, was enabled by a helium -jet tape transport system. The recommended yields in the evaluated data file are a combination of experimental and model-predicted values. The latter source is used since data from many short-lived fission products is still missing or poorly known. The results presented here, especially the ones for the very short-lived isotopes may be used to reduce the uncertainties associated with some of the existing values or to replace model-predicted yields. Gaussian distributions of elemental yields, based on the set of experimentally determined independent yields were examined. The feasibility of predicting unmeasured yields on the basis of charge and mass complementarity was also addressed.

  20. Consequences of extreme life history traits on population persistence: do short-lived gobies face demographic bottlenecks?

    NASA Astrophysics Data System (ADS)

    Lefèvre, Carine D.; Nash, Kirsty L.; González-Cabello, Alonso; Bellwood, David R.

    2016-06-01

    The majority of coral reef goby species are short-lived, with some highly abundant species living less than 100 d. To understand the role and consequences of this extreme life history in shaping coral reef fish populations, we quantitatively documented the structure of small reef fish populations over a 26-month period (>14 short-lived fish generations) at an inshore reef on the Great Barrier Reef, Australia. Most species with life spans >1 yr, such as pomacentrids, exhibited a peak in recruitment during the austral summer, driving seasonal changes in the small fish community composition. In contrast, there were no clear changes in goby community composition, despite the abundance of short-lived, high turnover species. Species of Eviota, the most abundant gobiid genus observed, showed remarkably similar demographic profiles year-round, with consistent densities of adults as well as recently recruited juveniles. Our results demonstrate ongoing recruitment of these small cryptic fishes, which appears to compensate for an exceptionally short life span on the reef. Our results suggest that gobiid populations are able to overcome demographic limitations, and by maintaining reproduction, larval survival and recruitment throughout the year, they may avoid population bottlenecks. These findings also underline the potential trophodynamic importance of these small species; because of this constant turnover, Eviota species and other short-lived fishes may be particularly valuable contributors to the flow of energy on coral reefs, underpinning the year-round trophic structure.

  1. A proposal for assessing study quality: Biomonitoring, Environmental Epidemiology, and Short-lived Chemicals (BEES-C) instrument.

    PubMed

    LaKind, Judy S; Sobus, Jon R; Goodman, Michael; Barr, Dana Boyd; Fürst, Peter; Albertini, Richard J; Arbuckle, Tye E; Schoeters, Greet; Tan, Yu-Mei; Teeguarden, Justin; Tornero-Velez, Rogelio; Weisel, Clifford P

    2014-12-01

    The quality of exposure assessment is a major determinant of the overall quality of any environmental epidemiology study. The use of biomonitoring as a tool for assessing exposure to ubiquitous chemicals with short physiologic half-lives began relatively recently. These chemicals present several challenges, including their presence in analytical laboratories and sampling equipment, difficulty in establishing temporal order in cross-sectional studies, short- and long-term variability in exposures and biomarker concentrations, and a paucity of information on the number of measurements required for proper exposure classification. To date, the scientific community has not developed a set of systematic guidelines for designing, implementing and interpreting studies of short-lived chemicals that use biomonitoring as the exposure metric or for evaluating the quality of this type of research for WOE assessments or for peer review of grants or publications. We describe key issues that affect epidemiology studies using biomonitoring data on short-lived chemicals and propose a systematic instrument--the Biomonitoring, Environmental Epidemiology, and Short-lived Chemicals (BEES-C) instrument--for evaluating the quality of research proposals and studies that incorporate biomonitoring data on short-lived chemicals. Quality criteria for three areas considered fundamental to the evaluation of epidemiology studies that include biological measurements of short-lived chemicals are described: 1) biomarker selection and measurement, 2) study design and execution, and 3) general epidemiological study design considerations. We recognize that the development of an evaluative tool such as BEES-C is neither simple nor non-controversial. We hope and anticipate that the instrument will initiate further discussion/debate on this topic. PMID:25137624

  2. A proposal for assessing study quality: Biomonitoring, Environmental Epidemiology, and Short-lived Chemicals (BEES-C) instrument

    PubMed Central

    LaKind, Judy S.; Sobus, Jon R.; Goodman, Michael; Barr, Dana Boyd; Fürst, Peter; Albertini, Richard J.; Arbuckle, Tye E.; Schoeters, Greet; Tan, Yu-Mei; Teeguarden, Justin; Tornero-Velez, Rogelio; Weisel, Clifford P.

    2015-01-01

    The quality of exposure assessment is a major determinant of the overall quality of any environmental epidemiology study. The use of biomonitoring as a tool for assessing exposure to ubiquitous chemicals with short physiologic half-lives began relatively recently. These chemicals present several challenges, including their presence in analytical laboratories and sampling equipment, difficulty in establishing temporal order in cross-sectional studies, short- and long-term variability in exposures and biomarker concentrations, and a paucity of information on the number of measurements required for proper exposure classification. To date, the scientific community has not developed a set of systematic guidelines for designing, implementing and interpreting studies of short-lived chemicals that use biomonitoring as the exposure metric or for evaluating the quality of this type of research for WOE assessments or for peer review of grants or publications. We describe key issues that affect epidemiology studies using biomonitoring data on short-lived chemicals and propose a systematic instrument – the Biomonitoring, Environmental Epidemiology, and Short-lived Chemicals (BEES-C) instrument – for evaluating the quality of research proposals and studies that incorporate biomonitoring data on short-lived chemicals. Quality criteria for three areas considered fundamental to the evaluation of epidemiology studies that include biological measurements of short-lived chemicals are described: 1) biomarker selection and measurement, 2) study design and execution, and 3) general epidemiological study design considerations. We recognize that the development of an evaluative tool such as BEES-C is neither simple nor non-controversial. We hope and anticipate that the instrument will initiate further discussion/debate on this topic. PMID:25137624

  3. Convective transport of very-short-lived bromocarbons to the stratosphere

    NASA Astrophysics Data System (ADS)

    Liang, Q.; Atlas, E.; Blake, D.; Dorf, M.; Pfeilsticker, K.; Schauffler, S.

    2014-01-01

    We use the NASA GEOS Chemistry Climate Model (GEOSCCM) to quantify the contribution of two most important brominated very short-lived substances (VSLS), bromoform (CHBr3) and dibromomethane (CH2Br2), to stratospheric bromine and its sensitivity to convection strength. Model simulations suggest that the most active transport of VSLS from the marine boundary layer through the tropopause occurs over the tropical Indian Ocean, the Western Pacific warm pool, and off the Pacific coast of Mexico. Together, convective lofting of CHBr3 and CH2Br2 and their degradation products supplies ∼8 ppt total bromine to the base of the Tropical Tropopause Layer (TTL, ∼150 hPa), similar to the amount of VSLS organic bromine available in the marine boundary layer (∼7.8-8.4 ppt) in the above active convective lofting regions. Of the total ∼8 ppt VSLS-originated bromine that enters the base of TTL at ∼150 hPa, half is in the form of source gas injection (SGI) and half as product gas injection (PGI). Only a small portion (< 10%) the VSLS-originated bromine is removed via wet scavenging in the TTL before reaching the lower stratosphere. On global and annual average, CHBr3 and CH2Br2, together, contribute ∼7.7 pptv to the present-day inorganic bromine in the stratosphere. However, varying model deep convection strength between maximum and minimum convection conditions can introduce a ∼2.6 pptv uncertainty in the contribution of VSLS to inorganic bromine in the stratosphere (BryVSLS). Contrary to the conventional wisdom, minimum convection condition leads to a larger BryVSLS as the reduced scavenging in soluble product gases, thus a significant increase in PGI (2-3 ppt), greatly exceeds the relative minor decrease in SGI (a few 10ths ppt).

  4. Convective Transport of Very-short-lived Bromocarbons to the Stratosphere

    NASA Technical Reports Server (NTRS)

    Liang, Qing; Atlas, Elliot Leonard; Blake, Donald Ray; Dorf, Marcel; Pfeilsticker, Klaus August; Schauffler, Sue Myhre

    2014-01-01

    We use the NASA GEOS Chemistry Climate Model (GEOSCCM) to quantify the contribution of two most important brominated very short-lived substances (VSLS), bromoform (CHBr3) and dibromomethane (CH2Br2), to stratospheric bromine and its sensitivity to convection strength. Model simulations suggest that the most active transport of VSLS from the marine boundary layer through the tropopause occurs over the tropical Indian Ocean, the Western Pacific warm pool, and off the Pacific coast of Mexico. Together, convective lofting of CHBr3 and CH2Br2 and their degradation products supplies 8 ppt total bromine to the base of the Tropical Tropopause Layer (TTL, 150 hPa), similar to the amount of VSLS organic bromine available in the marine boundary layer (7.8-8.4 ppt) in the above active convective lofting regions. Of the total 8 ppt VSLS-originated bromine that enters the base of TTL at 150 hPa, half is in the form of source gas injection (SGI) and half as product gas injection (PGI). Only a small portion (< 10%) the VSLS-originated bromine is removed via wet scavenging in the TTL before reaching the lower stratosphere. On global and annual average, CHBr3 and CH2Br2, together, contribute 7.7 pptv to the present-day inorganic bromine in the stratosphere. However, varying model deep convection strength between maximum and minimum convection conditions can introduce a 2.6 pptv uncertainty in the contribution of VSLS to inorganic bromine in the stratosphere (BryVSLS). Contrary to the conventional wisdom, minimum convection condition leads to a larger BryVSLS as the reduced scavenging in soluble product gases, thus a significant increase in PGI (2-3 ppt), greatly exceeds the relative minor decrease in SGI (a few 10ths ppt.

  5. MIXING AND TRANSPORT OF SHORT-LIVED AND STABLE ISOTOPES AND REFRACTORY GRAINS IN PROTOPLANETARY DISKS

    SciTech Connect

    Boss, Alan P.

    2013-08-10

    Analyses of primitive meteorites and cometary samples have shown that the solar nebula must have experienced a phase of large-scale outward transport of small refractory grains as well as homogenization of initially spatially heterogeneous short-lived isotopes. The stable oxygen isotopes, however, were able to remain spatially heterogeneous at the {approx}6% level. One promising mechanism for achieving these disparate goals is the mixing and transport associated with a marginally gravitationally unstable (MGU) disk, a likely cause of FU Orionis events in young low-mass stars. Several new sets of MGU models are presented that explore mixing and transport in disks with varied masses (0.016 to 0.13 M{sub Sun }) around stars with varied masses (0.1 to 1 M{sub Sun }) and varied initial Q stability minima (1.8 to 3.1). The results show that MGU disks are able to rapidly (within {approx}10{sup 4} yr) achieve large-scale transport and homogenization of initially spatially heterogeneous distributions of disk grains or gas. In addition, the models show that while single-shot injection heterogeneity is reduced to a relatively low level ({approx}1%), as required for early solar system chronometry, continuous injection of the sort associated with the generation of stable oxygen isotope fractionations by UV photolysis leads to a sustained, relatively high level ({approx}10%) of heterogeneity, in agreement with the oxygen isotope data. These models support the suggestion that the protosun may have experienced at least one FU Orionis-like outburst, which produced several of the signatures left behind in primitive chondrites and comets.

  6. Climate responses to anthropogenic emissions of short-lived climate pollutants

    NASA Astrophysics Data System (ADS)

    Baker, L. H.; Collins, W. J.; Olivié, D. J. L.; Cherian, R.; Hodnebrog, Ø.; Myhre, G.; Quaas, J.

    2015-07-01

    Policies to control air quality focus on mitigating emissions of aerosols and their precursors, and other short-lived climate pollutants (SLCPs). On a local scale, these policies will have beneficial impacts on health and crop yields, by reducing particulate matter (PM) and surface ozone concentrations; however, the climate impacts of reducing emissions of SLCPs are less straightforward to predict. In this paper we consider a set of idealized, extreme mitigation strategies, in which the total anthropogenic emissions of individual SLCP emissions species are removed. This provides an upper bound on the potential climate impacts of such air quality strategies. We focus on evaluating the climate responses to changes in anthropogenic emissions of aerosol precursor species: black carbon (BC), organic carbon (OC) and sulphur dioxide (SO2). We perform climate integrations with four fully coupled atmosphere-ocean global climate models (AOGCMs), and examine the effects on global and regional climate of removing the total land-based anthropogenic emissions of each of the three aerosol precursor species. We find that the SO2 emissions reductions lead to the strongest response, with all models showing an increase in surface temperature focussed in the Northern Hemisphere mid and (especially) high latitudes, and showing a corresponding increase in global mean precipitation. Changes in precipitation patterns are driven mostly by a northward shift in the ITCZ (Intertropical Convergence Zone), consistent with the hemispherically asymmetric warming pattern driven by the emissions changes. The BC and OC emissions reductions give a much weaker response, and there is some disagreement between models in the sign of the climate responses to these perturbations. These differences between models are due largely to natural variability in sea-ice extent, circulation patterns and cloud changes. This large natural variability component to the signal when the ocean circulation and sea-ice are

  7. Climate responses to anthropogenic emissions of short-lived climate pollutants

    NASA Astrophysics Data System (ADS)

    Baker, L. H.; Collins, W. J.; Olivié, D. J. L.; Cherian, R.; Hodnebrog, Ø.; Myhre, G.; Quaas, J.; Samset, B. H.

    2015-02-01

    Policies to control air quality focus on mitigating emissions of aerosols and their precursors, and other short-lived climate pollutants (SLCPs). On a local scale, these policies will have beneficial impacts on health and crop yields, by reducing particulate matter (PM) and surface ozone concentrations; however, the climate impacts of reducing emissions of SLCPs are less straightforward to predict. In this paper we consider a set of idealised, extreme mitigation strategies, in which the total anthropogenic emissions of individual SLCP emissions species are removed. This provides an upper bound on the potential climate impacts of such air quality strategies. We focus on evaluating the climate responses to changes in anthropogenic emissions of aerosol precursor species: black carbon (BC), organic carbon (OC) and sulphur dioxide (SO2). We perform climate integrations with four fully coupled atmosphere-ocean global climate models (AOGCMs), and examine the effects on global and regional climate of removing the total land-based anthropogenic emissions of each of the three aerosol precursor species. We find that the SO2 emissions reductions lead to the strongest response, with all three models showing an increase in surface temperature focussed in the northern hemisphere high latitudes, and a corresponding increase in global mean precipitation and run-off. Changes in precipitation and run-off patterns are driven mostly by a northward shift in the ITCZ, consistent with the hemispherically asymmetric warming pattern driven by the emissions changes. The BC and OC emissions reductions give a much weaker forcing signal, and there is some disagreement between models in the sign of the climate responses to these perturbations. These differences between models are due largely to natural variability in sea-ice extent, circulation patterns and cloud changes. This large natural variability component to the signal when the ocean circulation and sea-ice are free-running means that the

  8. Response of Arctic temperature to changes in emissions of short-lived climate forcers

    NASA Astrophysics Data System (ADS)

    Sand, M.; Berntsen, T. K.; von Salzen, K.; Flanner, M. G.; Langner, J.; Victor, D. G.

    2016-03-01

    There is growing scientific and political interest in the impacts of climate change and anthropogenic emissions on the Arctic. Over recent decades temperatures in the Arctic have increased at twice the global rate, largely as a result of ice-albedo and temperature feedbacks. Although deep cuts in global CO2 emissions are required to slow this warming, there is also growing interest in the potential for reducing short-lived climate forcers (SLCFs; refs ,). Politically, action on SLCFs may be particularly promising because the benefits of mitigation are seen more quickly than for mitigation of CO2 and there are large co-benefits in terms of improved air quality. This Letter is one of the first to systematically quantify the Arctic climate impact of regional SLCFs emissions, taking into account black carbon (BC), sulphur dioxide (SO2), nitrogen oxides (NOx), volatile organic compounds (VOCs), organic carbon (OC) and tropospheric ozone (O3), and their transport processes and transformations in the atmosphere. This study extends the scope of previous works by including more detailed calculations of Arctic radiative forcing and quantifying the Arctic temperature response. We find that the largest Arctic warming source is from emissions within the Asian nations owing to the large absolute amount of emissions. However, the Arctic is most sensitive, per unit mass emitted, to SLCFs emissions from a small number of activities within the Arctic nations themselves. A stringent, but technically feasible mitigation scenario for SLCFs, phased in from 2015 to 2030, could cut warming by 0.2 (+/-0.17) K in 2050.

  9. Response of Arctic Temperature to Changes in Emissions of Short-Lived Climate Forcers

    NASA Astrophysics Data System (ADS)

    Sand, M.; Berntsen, T.; von Salzen, K.; Flanner, M.; Langner, J.; Victor, D. G.

    2014-12-01

    There is growing scientific and political interest in the impacts of climate change and anthropogenic emissions on the Arctic. Over recent decades temperatures in the Arctic have increased twice the global rate, largely due to ice albedo and temperature feedbacks. While deep cuts in global CO2 emissions are required to slow this warming, there is also growing interest in the potential for reducing short lived climate forcers (SLCFs). Politically, action on SLCFs may be particularly promising because the benefits of mitigation appear promptly and there are large co-benefits in terms of improved air quality. This study is the first to systematically quantify the Arctic climate impact of regional SLCF emissions, taking into account BC, sulphur dioxide (SO2), nitrogen oxides (NOx), volatile hydrocarbons (VOC), organic carbon (OC) and tropospheric ozone, their transport processes and transformations in the atmosphere. Using several chemical transport models we perform detailed radiative forcing calculations from emissions of these species. Geographically we separate emissions into seven source regions that correspond with the national groupings of the Arctic Council, the leading body organizing international policy in the region (the United States, Canada, the Nordic countries, the rest of Europe, Russia, East and South Asia, and the rest of the world). We look at six main sectors known to account for [nearly all] of these emissions: households (domestic), energy/industry/waste, transport, agricultural fires, grass/forest fires, and gas flaring. We find that the largest Arctic warming source is from emissions within the Asian nations. However, the Arctic is most sensitive, per unit mass emitted, to SLCFs emissions from a small number of activities within the Arctic nations themselves. A stringent, but technically feasible SLCFs mitigation scenario, phased in from 2015 through 2030, can cut warming by 0.2 K in 2050.

  10. Treatment of solid tumors by interstitial release of recoiling short-lived alpha emitters

    NASA Astrophysics Data System (ADS)

    Arazi, L.; Cooks, T.; Schmidt, M.; Keisari, Y.; Kelson, I.

    2007-08-01

    A new method utilizing alpha particles to treat solid tumors is presented. Tumors are treated with interstitial radioactive sources which continually release short-lived alpha emitting atoms from their surface. The atoms disperse inside the tumor, delivering a high dose through their alpha decays. We implement this scheme using thin wire sources impregnated with 224Ra, which release by recoil 220Rn, 216Po and 212Pb atoms. This work aims to demonstrate the feasibility of our method by measuring the activity patterns of the released radionuclides in experimental tumors. Sources carrying 224Ra activities in the range 10-130 kBq were used in experiments on murine squamous cell carcinoma tumors. These included gamma spectroscopy of the dissected tumors and major organs, Fuji-plate autoradiography of histological tumor sections and tissue damage detection by Hematoxylin-Eosin staining. The measurements focused on 212Pb and 212Bi. The 220Rn/216Po distribution was treated theoretically using a simple diffusion model. A simplified scheme was used to convert measured 212Pb activities to absorbed dose estimates. Both physical and histological measurements confirmed the formation of a 5-7 mm diameter necrotic region receiving a therapeutic alpha-particle dose around the source. The necrotic regions shape closely corresponded to the measured activity patterns. 212Pb was found to leave the tumor through the blood at a rate which decreased with tumor mass. Our results suggest that the proposed method, termed DART (diffusing alpha-emitters radiation therapy), may potentially be useful for the treatment of human patients.

  11. Higher Accuracy Measurements of Photochemical Properties of Very Short-Lived Substances.

    NASA Astrophysics Data System (ADS)

    Orkin, V. L.; Khamaganov, V. G.; Kurylo, M. J., III

    2015-12-01

    Despite the broad applicability of simple fully halogenated hydrocarbons in various industries, the production and use of bromo(chloro)fluorocarbons (Halons) and chlorofluorocarbons (CFCs) has been phased out because of the danger they pose to the Earth's stratospheric ozone layer. In addition, all halogen-containing hydrocarbons are infrared active gases because of their strong absorption bands in the region of the atmospheric transparency window between ca. 8 and 12 mm that can affect the Earth's radiation balance. However, the effort to find replacements continues to return to bromine (chlorine)-containing compounds because of their excellent properties as industrial solvents and cleaning agents and especially because of bromine efficiency as a chemically active flame suppressant. The primary approach to this problem has been to test candidate replacement compounds that have very short atmospheric lifetimes and therefore substantially reduced ozone depleting and radiative impacts. Reactions with hydroxyl radicals (OH) and photolysis are the main processes dictating the compound residence time in the atmosphere for a majority of trace gases. In case of very short-lived substances (VSLS) their reaction with OH dictates both the atmospheric lifetime and active halogen release. Therefore, the accuracy of OH kinetic data is of primary importance for the purpose of comprehensive atmospheric modeling of compound's impact on the atmosphere, such as in ozone depletion and climate change. We demonstrated the ability to determine the OH reaction rate constants over the temperature range of atmospheric interest with the total uncertainty of ~2-3%, thus making laboratory measurements a negligible source of uncertainty in atmospheric modeling. These studies revealed the different reactivity of molecular isomers toward OH and a non-Arrhenius behavior of the temperature dependence to be a rather common kinetic feature of the OH reactivity, which can be accounted for in

  12. Disentangling the effects of CO2 and short-lived climate forcer mitigation.

    PubMed

    Rogelj, Joeri; Schaeffer, Michiel; Meinshausen, Malte; Shindell, Drew T; Hare, William; Klimont, Zbigniew; Velders, Guus J M; Amann, Markus; Schellnhuber, Hans Joachim

    2014-11-18

    Anthropogenic global warming is driven by emissions of a wide variety of radiative forcers ranging from very short-lived climate forcers (SLCFs), like black carbon, to very long-lived, like CO2. These species are often released from common sources and are therefore intricately linked. However, for reasons of simplification, this CO2-SLCF linkage was often disregarded in long-term projections of earlier studies. Here we explicitly account for CO2-SLCF linkages and show that the short- and long-term climate effects of many SLCF measures consistently become smaller in scenarios that keep warming to below 2 °C relative to preindustrial levels. Although long-term mitigation of methane and hydrofluorocarbons are integral parts of 2 °C scenarios, early action on these species mainly influences near-term temperatures and brings small benefits for limiting maximum warming relative to comparable reductions taking place later. Furthermore, we find that maximum 21st-century warming in 2 °C-consistent scenarios is largely unaffected by additional black-carbon-related measures because key emission sources are already phased-out through CO2 mitigation. Our study demonstrates the importance of coherently considering CO2-SLCF coevolutions. Failing to do so leads to strongly and consistently overestimating the effect of SLCF measures in climate stabilization scenarios. Our results reinforce that SLCF measures are to be considered complementary rather than a substitute for early and stringent CO2 mitigation. Near-term SLCF measures do not allow for more time for CO2 mitigation. We disentangle and resolve the distinct benefits across different species and therewith facilitate an integrated strategy for mitigating both short and long-term climate change. PMID:25368182

  13. Response of Arctic Temperature to Changes in Emissions of Short-Lived Climate Forcers

    NASA Astrophysics Data System (ADS)

    Sand, M.; Berntsen, T.; von Salzen, K.; Flanner, M.; Langner, J.; Victor, D. G.

    2015-12-01

    There is growing scientific and political interest in the impacts of climate change and anthropogenic emissions on the Arctic. Over recent decades temperatures in the Arctic have increased twice the global rate, largely due to ice albedo and temperature feedbacks. While deep cuts in global CO2 emissions are required to slow this warming, there is also growing interest in the potential for reducing short lived climate forcers (SLCFs). Politically, action on SLCFs may be particularly promising because the benefits of mitigation appear promptly and there are large co-benefits in terms of improved air quality. This study is the first to systematically quantify the Arctic climate impact of regional SLCF emissions, taking into account BC, sulphur dioxide (SO2), nitrogen oxides (NOx), volatile hydrocarbons (VOC), organic carbon (OC) and tropospheric ozone, their transport processes and transformations in the atmosphere. Using several chemical transport models we perform detailed radiative forcing calculations from emissions of these species. Geographically we separate emissions into seven source regions that correspond with the national groupings of the Arctic Council, the leading body organizing international policy in the region (the United States, Canada, the Nordic countries, the rest of Europe, Russia, East and South Asia, and the rest of the world). We look at six main sectors known to account for [nearly all] of these emissions: households (domestic), energy/industry/waste, transport, agricultural fires, grass/forest fires, and gas flaring. We find that the largest Arctic warming source is from emissions within the Asian nations. However, the Arctic is most sensitive, per unit mass emitted, to SLCFs emissions from a small number of activities within the Arctic nations themselves. A stringent, but technically feasible SLCFs mitigation scenario, phased in from 2015 through 2030, can cut warming by 0.2 K in 2050.

  14. Large Differences in Aging Phenotype between Strains of the Short-Lived Annual Fish Nothobranchius furzeri

    PubMed Central

    Benedetti, Mauro; Roncaglia, Paola; Cattaneo, Antonino; Domenici, Luciano; Cellerino, Alessandro

    2008-01-01

    Background A laboratory inbred strain of the annual fish Nothobranchius furzeri shows exceptionally short life expectancy and accelerated expression of age markers. In this study, we analyze new wild-derived lines of this short-lived species. Methodology/Principal Findings We characterized captive survival and age-related traits in F1 and F2 offspring of wild-caught N. furzeri. Wild-derived N. furzeri lines showed expression of lipofuscin and neurodegeneration at age 21 weeks. Median lifespan in the laboratory varied from to 20 to 23 weeks and maximum lifespan from 25 to 32 weeks. These data demonstrate that rapid age-dependent decline and short lifespan are natural characteristics of this species. The N. furzeri distribution range overlaps with gradients in altitude and aridity. Fish from more arid habitats are expected to experience a shorter survival window in the wild. We tested whether captive lines stemming from semi-arid and sub-humid habitats differ in longevity and expression of age-related traits. We detected a clear difference in age-dependent cognitive decline and a slight difference in lifespan (16% for median, 15% for maximum lifespan) between these lines. Finally, we observed shorter lifespan and accelerated expression of age-related markers in the inbred laboratory strain compared to these wild-derived lines. Conclusions/Significance Owing to large differences in aging phenotypes in different lines, N. furzeri could represent a model system for studying the genetic control of life-history traits in natural populations. PMID:19052641

  15. Multimodel emission metrics for regional emissions of short lived climate forcers

    NASA Astrophysics Data System (ADS)

    Aamaas, B.; Berntsen, T. K.; Fuglestvedt, J. S.; Shine, K. P.; Bellouin, N.

    2015-09-01

    For short lived climate forcers (SLCFs), the impact of emissions depends on where and when the emissions take place. Comprehensive new calculations of various emission metrics for SLCFs are presented based on radiative forcing (RF) values calculated in four different (chemistry-transport or coupled-chemistry climate) models. We distinguish between emissions during summer (May-October) and winter season (November-April) for emissions from Europe, East Asia, as well as the global shipping sector. The species included in this study are aerosols and aerosols precursors (BC, OC, SO2, NH3), and ozone precursors (NOx, CO, VOC), which also influence aerosols, to a lesser degree. Emission metrics for global climate responses of these emissions, as well as for CH4, have been calculated relative to CO2, using Global Warming Potential (GWP) and Global Temperature change Potential (GTP), based on dedicated RF simulations by four global models. The emission metrics include indirect cloud effects of aerosols and the semi-direct forcing for BC. In addition to the standard emission metrics for pulse and sustained emissions, we have also calculated a new emission metric designed for an emission profile consisting of a ramp up period of 15 years followed by sustained emissions, which is more appropriate for a gradual implementation of mitigation policies. For the aerosols, the emission metric values are larger in magnitude for Europe than East Asia and for summer than winter. A variation is also observed for the ozone precursors, with largest values in East Asia and winter for CO and in Europe and summer for VOC. In general, the variations between the emission metrics derived from different models are larger than the variations between regions and seasons, but the regional and seasonal variations for the best estimate also hold for most of the models individually. Further, the estimated climate impact of a mitigation policy package is robust even when accounting for correlations. For

  16. Regional emission metrics for short-lived climate forcers from multiple models

    NASA Astrophysics Data System (ADS)

    Aamaas, Borgar; Berntsen, Terje K.; Fuglestvedt, Jan S.; Shine, Keith P.; Bellouin, Nicolas

    2016-06-01

    For short-lived climate forcers (SLCFs), the impact of emissions depends on where and when the emissions take place. Comprehensive new calculations of various emission metrics for SLCFs are presented based on radiative forcing (RF) values calculated in four different (chemical-transport or coupled chemistry-climate) models. We distinguish between emissions during summer (May-October) and winter (November-April) for emissions in Europe and East Asia, as well as from the global shipping sector and global emissions. The species included in this study are aerosols and aerosol precursors (BC, OC, SO2, NH3), as well as ozone precursors (NOx, CO, VOCs), which also influence aerosols to a lesser degree. Emission metrics for global climate responses of these emissions, as well as for CH4, have been calculated using global warming potential (GWP) and global temperature change potential (GTP), based on dedicated RF simulations by four global models. The emission metrics include indirect cloud effects of aerosols and the semi-direct forcing for BC. In addition to the standard emission metrics for pulse and sustained emissions, we have also calculated a new emission metric designed for an emission profile consisting of a ramping period of 15 years followed by sustained emissions, which is more appropriate for a gradual implementation of mitigation policies.For the aerosols, the emission metric values are larger in magnitude for emissions in Europe than East Asia and for summer than winter. A variation is also observed for the ozone precursors, with largest values for emissions in East Asia and winter for CO and in Europe and summer for VOCs. In general, the variations between the emission metrics derived from different models are larger than the variations between regions and seasons, but the regional and seasonal variations for the best estimate also hold for most of the models individually. Further, the estimated climate impact of an illustrative mitigation policy package is

  17. Evaluating the climate and air quality impacts of short-lived pollutants

    NASA Astrophysics Data System (ADS)

    Stohl, A.; Aamaas, B.; Amann, M.; Baker, L. H.; Bellouin, N.; Berntsen, T. K.; Boucher, O.; Cherian, R.; Collins, W.; Daskalakis, N.; Dusinska, M.; Eckhardt, S.; Fuglestvedt, J. S.; Harju, M.; Heyes, C.; Hodnebrog, Ø.; Hao, J.; Im, U.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Law, K. S.; Lund, M. T.; Maas, R.; MacIntosh, C. R.; Myhre, G.; Myriokefalitakis, S.; Olivié, D.; Quaas, J.; Quennehen, B.; Raut, J.-C.; Rumbold, S. T.; Samset, B. H.; Schulz, M.; Seland, Ø.; Shine, K. P.; Skeie, R. B.; Wang, S.; Yttri, K. E.; Zhu, T.

    2015-06-01

    This paper presents a summary of the work done within the European Union's Seventh Framework Programme project ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants). ECLIPSE had a unique systematic concept for designing a realistic and effective mitigation scenario for short-lived climate pollutants (SLCPs: methane, aerosols and ozone, and their precursor species) and quantifying its climate and air quality impacts, and this paper presents the results in the context of this overarching strategy. The first step in ECLIPSE was to create a new emission inventory based on current legislation (CLE) for the recent past and until 2050. Substantial progress compared to previous work was made by including previously unaccounted types of sources such as flaring of gas associated with oil production, and wick lamps. These emission data were used for present-day reference simulations with four advanced Earth system models (ESMs) and six chemistry transport models (CTMs). The model simulations were compared with a variety of ground-based and satellite observational data sets from Asia, Europe and the Arctic. It was found that the models still underestimate the measured seasonality of aerosols in the Arctic but to a lesser extent than in previous studies. Problems likely related to the emissions were identified for Northern Russia and India, in particular. To estimate the climate impacts of SLCPs, ECLIPSE followed two paths of research: the first path calculated radiative forcing (RF) values for a large matrix of SLCP species emissions, for different seasons and regions independently. Based on these RF calculations, the Global Temperature change Potential metric for a time horizon of 20 years (GTP20) was calculated for each SLCP emission type. This climate metric was then used in an integrated assessment model to identify all emission mitigation measures with a beneficial air quality and short-term (20 year) climate impact. These measures together

  18. Evaluating the climate and air quality impacts of short-lived pollutants

    NASA Astrophysics Data System (ADS)

    Stohl, A.; Aamaas, B.; Amann, M.; Baker, L. H.; Bellouin, N.; Berntsen, T. K.; Boucher, O.; Cherian, R.; Collins, W.; Daskalakis, N.; Dusinska, M.; Eckhardt, S.; Fuglestvedt, J. S.; Harju, M.; Heyes, C.; Hodnebrog, Ø.; Hao, J.; Im, U.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Law, K. S.; Lund, M. T.; Maas, R.; MacIntosh, C. R.; Myhre, G.; Myriokefalitakis, S.; Olivié, D.; Quaas, J.; Quennehen, B.; Raut, J.-C.; Rumbold, S. T.; Samset, B. H.; Schulz, M.; Seland, Ø.; Shine, K. P.; Skeie, R. B.; Wang, S.; Yttri, K. E.; Zhu, T.

    2015-09-01

    This paper presents a summary of the work done within the European Union's Seventh Framework Programme project ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants). ECLIPSE had a unique systematic concept for designing a realistic and effective mitigation scenario for short-lived climate pollutants (SLCPs; methane, aerosols and ozone, and their precursor species) and quantifying its climate and air quality impacts, and this paper presents the results in the context of this overarching strategy. The first step in ECLIPSE was to create a new emission inventory based on current legislation (CLE) for the recent past and until 2050. Substantial progress compared to previous work was made by including previously unaccounted types of sources such as flaring of gas associated with oil production, and wick lamps. These emission data were used for present-day reference simulations with four advanced Earth system models (ESMs) and six chemistry transport models (CTMs). The model simulations were compared with a variety of ground-based and satellite observational data sets from Asia, Europe and the Arctic. It was found that the models still underestimate the measured seasonality of aerosols in the Arctic but to a lesser extent than in previous studies. Problems likely related to the emissions were identified for northern Russia and India, in particular. To estimate the climate impacts of SLCPs, ECLIPSE followed two paths of research: the first path calculated radiative forcing (RF) values for a large matrix of SLCP species emissions, for different seasons and regions independently. Based on these RF calculations, the Global Temperature change Potential metric for a time horizon of 20 years (GTP20) was calculated for each SLCP emission type. This climate metric was then used in an integrated assessment model to identify all emission mitigation measures with a beneficial air quality and short-term (20-year) climate impact. These measures together

  19. Evaluating the climate and air quality impacts of short-lived pollutants

    NASA Astrophysics Data System (ADS)

    Stohl, A.; Aamaas, B.; Amann, M.; Baker, L. H.; Bellouin, N.; Berntsen, T. K.; Boucher, O.; Cherian, R.; Collins, W.; Daskalakis, N.; Dusinska, M.; Eckhardt, S.; Fuglestvedt, J. S.; Harju, M.; Heyes, C.; Hodnebrog, Ø.; Hao, J.; Im, U.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Law, K. S.; Lund, M. T.; Maas, R.; MacIntosh, C. R.; Myhre, G.; Myriokefalitakis, S.; Olivié, D.; Quaas, J.; Quennehen, B.; Raut, J.-C.; Rumbold, S. T.; Samset, B. H.; Schulz, M.; Seland, Ø.; Shine, K. P.; Skeie, R. B.; Wang, S.; Yttri, K. E.; Zhu, T.

    2015-06-01

    This paper presents a summary of the work done within the European Union's Seventh Framework Programme project ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants). ECLIPSE had a unique systematic concept for designing a realistic and effective mitigation scenario for short-lived climate pollutants (SLCPs: methane, aerosols and ozone, and their precursor species) and quantifying its climate and air quality impacts, and this paper presents the results in the context of this overarching strategy. The first step in ECLIPSE was to create a new emission inventory based on current legislation (CLE) for the recent past and until 2050. Substantial progress compared to previous work was made by including previously unaccounted types of sources such as flaring of gas associated with oil production, and wick lamps. These emission data were used for present-day reference simulations with four advanced Earth system models (ESMs) and six chemistry transport models (CTMs). The model simulations were compared with a variety of ground-based and satellite observational data sets from Asia, Europe and the Arctic. It was found that the models still underestimate the measured seasonality of aerosols in the Arctic but to a lesser extent than in previous studies. Problems likely related to the emissions were identified for Northern Russia and India, in particular. To estimate the climate impacts of SLCPs, ECLIPSE followed two paths of research: the first path calculated radiative forcing (RF) values for a large matrix of SLCP species emissions, for different seasons and regions independently. Based on these RF calculations, the Global Temperature change Potential metric for a time horizon of 20 years (GTP20) was calculated for each SLCP emission type. This climate metric was then used in an integrated assessment model to identify all emission mitigation measures with a beneficial air quality and short-term (20 year) climate impact. These measures together

  20. Evaluating the climate and air quality impacts of short-lived pollutants

    NASA Astrophysics Data System (ADS)

    Stohl, A.; Aamaas, B.; Amann, M.; Baker, L. H.; Bellouin, N.; Berntsen, T. K.; Boucher, O.; Cherian, R.; Collins, W.; Daskalakis, N.; Dusinska, M.; Eckhardt, S.; Fuglestvedt, J. S.; Harju, M.; Heyes, C.; Hodnebrog, Ø.; Hao, J.; Im, U.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Law, K. S.; Lund, M. T.; Maas, R.; MacIntosh, C. R.; Myhre, G.; Myriokefalitakis, S.; Olivié, D.; Quaas, J.; Quennehen, B.; Raut, J.-C.; Rumbold, S. T.; Samset, B. H.; Schulz, M.; Seland, Ø.; Shine, K. P.; Skeie, R. B.; Wang, S.; Yttri, K. E.; Zhu, T.

    2015-09-01

    This paper presents a summary of the work done within the European Union's Seventh Framework Programme project ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants). ECLIPSE had a unique systematic concept for designing a realistic and effective mitigation scenario for short-lived climate pollutants (SLCPs; methane, aerosols and ozone, and their precursor species) and quantifying its climate and air quality impacts, and this paper presents the results in the context of this overarching strategy. The first step in ECLIPSE was to create a new emission inventory based on current legislation (CLE) for the recent past and until 2050. Substantial progress compared to previous work was made by including previously unaccounted types of sources such as flaring of gas associated with oil production, and wick lamps. These emission data were used for present-day reference simulations with four advanced Earth system models (ESMs) and six chemistry transport models (CTMs). The model simulations were compared with a variety of ground-based and satellite observational data sets from Asia, Europe and the Arctic. It was found that the models still underestimate the measured seasonality of aerosols in the Arctic but to a lesser extent than in previous studies. Problems likely related to the emissions were identified for northern Russia and India, in particular. To estimate the climate impacts of SLCPs, ECLIPSE followed two paths of research: the first path calculated radiative forcing (RF) values for a large matrix of SLCP species emissions, for different seasons and regions independently. Based on these RF calculations, the Global Temperature change Potential metric for a time horizon of 20 years (GTP20) was calculated for each SLCP emission type. This climate metric was then used in an integrated assessment model to identify all emission mitigation measures with a beneficial air quality and short-term (20-year) climate impact. These measures together

  1. SU-C-204-07: The Production of Short-Lived Positron Emitters in Proton Therapy

    SciTech Connect

    Buitenhuis, H J T; Dendooven, P; Biegun, A K; Goethem, M-J van; Graaf, E R van der; Brandenburg, S; Diblen, F

    2015-06-15

    Purpose: To investigate the production and effect of short-lived positron emitters when using PET for in-vivo range verification during a proton therapy irradiation. Methods: The integrated production of short-lived positron emitters in the stopping of 55 MeV protons was measured in water, carbon, phosphorus and calcium targets. The experimental production rates are used to calculate the production on PMMA and a representative set of 4 tissue materials. The number of decays integrated over an irradiation in these materials is calculated as function of the duration of the irradiation, considering irradiations with the same total number of protons. Results: The most copiously produced short-lived nuclides and their production rates relative to the relevant long-lived nuclides are: 12-N (T1/2 = 11 ms) on carbon (9.5% of the 11-C production), 29-P (T1/2 = 4.1 s) on phosphorus (20% of the 30-P production) and 38m-K (T1/2 = 0.92 s) on calcium (113% of the 38g-K production). No short-lived nuclides are produced on water. The most noticeable Result is that for an irradiation in (carbon-rich) adipose tissue, 12-N will dominate the PET image up to an irradiation duration of 70 s. On bone tissue, 15-O dominates over 12-N after 7–15 s (depending on the carbon-to-oxygen ratio). Conclusions: The presence of 12-N needs to be considered in PET imaging during proton beam irradiations as, depending on tissue composition and PET scanning protocol, it may noticeably deteriorate image quality due to the large positron range blurring. The results presented warrant investigations into the energy-dependent production of 12-N, 29-P and 38m-K and their effect on PET imaging during proton irradiations.

  2. Short-lived chlorine-36 in a Ca- and Al-rich inclusion from the Ningqiang carbonaceous chondrite.

    PubMed

    Lin, Yangting; Guan, Yunbin; Leshin, Laurie A; Ouyang, Ziyuan; Wang, Daode

    2005-02-01

    Excesses of sulfur-36 in sodalite, a chlorine-rich mineral, in a calcium- and aluminum-rich inclusion from the Ningqiang carbonaceous chondrite linearly correlate with chorine/sulfur ratios, providing direct evidence for the presence of short-lived chlorine-36 (with a half-life of 0.3 million years) in the early solar system. The best inferred (36Cl/35Cl)o ratios of the sodalite are approximately 5 x 10(-6). Different from other short-lived radionuclides, chlorine-36 was introduced into the inclusion by solid-gas reaction during secondary alteration. The alteration reaction probably took place at least 1.5 million years after the first formation of the inclusion, based on the correlated study of the 26Al-26Mg systems of the relict primary minerals and the alteration assemblages, from which we inferred an initial ratio of (36Cl/35Cl)o > or = 1.6 x 10(-4) at the time when calcium- and aluminum-rich inclusions formed. This discovery supports a supernova origin of short-lived nuclides [Cameron, A. G. W., Hoeflich, P., Myers, P. C. & Clayton, D. D. (1995) Astrophys. J. 447, L53; Wasserburg, G. J., Gallino, R. & Busso, M. (1998) Astrophys. J. 500, L189-L193], but presents a serious challenge for local irradiation models [Shu, F. H., Shang, H., Glassgold, A. E. & Lee, T. (1997) Science 277, 1475-1479; Gounelle, M., Shu, F. H., Shang, H., Glassgold, A. E., Rehm, K. E. & Lee, T. (2001) Astrophys. J. 548, 1051-1070]. Furthermore, the short-lived 36Cl may serve as a unique fine-scale chronometer for volatile-rock interaction in the early solar system because of its close association with aqueous and/or anhydrous alteration processes. PMID:15671168

  3. Life-history variation in the short-lived herb Rorippa palustris: The role of carbon storage

    NASA Astrophysics Data System (ADS)

    Sosnová, Monika; Klimešová, Jitka

    2009-09-01

    Carbon storage is commonly found among perennials, but only rarely in annuals. However, many short-lived species may behave as annuals or short-lived perennials depending on the date of germination, photoperiod or disturbance. Due to the trade-off between investments into current reproduction vs. survival, these life-history modes presumably differ in carbon allocation. In this study, we aimed to evaluate how carbon storage is affected by germination date and disturbance in an outdoor pot experiment with the short-lived Rorippa palustris. Plants from autumnal and summer cohorts were injured in different ontogenetic stages (vegetative, flowering and fruiting) and the starch content in roots was assessed. Plants from the autumnal cohort invested more carbon into growth and reproduction, whereas plants from the summer cohort invested preferentially into reserves. However, injury changed the allocation pattern: in plants from the autumnal cohort, injury prevented allocation to reproduction and thus injured plants had a larger carbon storage at the end of the season than control plants; injury at the flowering and fruiting stage caused depletion of reserves for regrowth in plants from the summer cohort, resulting in lower starch reserves compared to control plants. We suggest that life-history variation in R. palustris can be caused by changes in its carbon economy: when all resources could not be used for flowering due to weak photoinduction or loss of flowering organs due to injury, part of the resources is stored for over wintering and reproduction in the next year.

  4. Beta-decay half-lives for the r-process nuclei

    NASA Astrophysics Data System (ADS)

    Panov, I. V.; Lutostansky, Yu. S.; Thielemann, F.-K.

    2016-03-01

    For nucleosynthesis calculations of the r-process it is important to know beta-decay half-lives of short-lived neutron-rich nuclei. In the present paper these characteristics are calculated for an extended number of neutron-rich nuclei, important for the r-process. In our calculations the model description of beta-strength functions based on Finite Fermi-Systems Theory is used. The comparison with other predictions and experimental data is done. It is shown that the accuracy of beta-decay half-lives of short-lived neutron-rich nuclei is increasing with increasing neutron excess and can be used for modeling of nucleosynthesis of heavy nuclei in the r-process. For nuclei heavier than lead the half-lives of neutron-rich nuclei are on average 10 times smaller, than proposed of other predictions.

  5. Probing the Collective Degrees of Freedom at the Proton Drip Line in the Extremely Neutron Deficient {sup 172}Hg

    SciTech Connect

    Sandzelius, M.; Cederwall, B.; Hadinia, B.; Andgren, K.; Baeck, T.; Johnson, A.; Khaplanov, A.; Wyss, R.; Ganioglu, E.; Grahn, T.; Greenlees, P. T.; Jakobsson, U.; Jones, P. M.; Julin, R.; Juutinen, S.; Ketelhut, S.; Leino, M.; Nyman, M.; Peura, P.; Rahkila, P.; and others

    2011-11-30

    Excited states in the extremely neutron-deficient isotope {sup 172}Hg have been established for the first time. The {sup 96}Ru({sup 78}Kr,2n) reaction was employed to populate excited states in {sup 172}Hg with a cross section {sigma}{approx_equal} 15 nb. The highly selective Recoil-Decay Tagging (RDT) technique was used to obtain clean in-beam {gamma}-ray spectra for {sup 172}Hg. The yrast ground-state band has tentatively been established up to I = 6h-bar. The data have been interpreted within the framework of total Routhian surface and quasiparticle random phase approximation calculations. In addition to the well-known features of shape coexistence previously observed in light Hg isotopes, the systematic trends in the energy of the yrast 2{sup +} and 4{sup +} states in the chain of Hg isotopes indicate a pronounced vibrational collectivity which is reduced in strength, but at the same time shows a higher degree of harmonicity, as the neutron number decreases below the neutron midshell.

  6. Isospin symmetry in the s d shell: Transition strengths in the neutron-deficient s d shell nucleus 33Ar

    NASA Astrophysics Data System (ADS)

    Wendt, A.; Taprogge, J.; Reiter, P.; Golubev, P.; Grawe, H.; Pietri, S.; Boutachkov, P.; Algora, A.; Ameil, F.; Bentley, M. A.; Blazhev, A.; Bloor, D.; Bondili, N. S.; Bowry, M.; Bracco, A.; Braun, N.; Camera, F.; Cederkäll, J.; Crespi, F.; de la Salle, A.; DiJulio, D.; Doornenbal, P.; Geibel, K.; Gellanki, J.; Gerl, J.; GrÈ©bosz, J.; Guastalla, G.; Habermann, T.; Hackstein, M.; Hoischen, R.; Jungclaus, A.; Merchán, E.; Million, B.; Morales, A.; Moschner, K.; Podolyák, Zs.; Pietralla, N.; Ralet, D.; Reese, M.; Rudolph, D.; Scruton, L.; Siebeck, B.; Warr, N.; Wieland, O.; Wollersheim, H. J.

    2014-11-01

    Reduced transition strengths of the deexciting transitions from the first two excited states in 33Ar were measured in a relativistic Coulomb excitation experiment at the GSI Helmholtz center. The radioactive ion beam was produced by fragmentation of a primary 36Ar beam on a 9Be target followed by the selection of the reaction product of interest via the GSI Fragment Separator. The 33Ar beam hit a secondary 197Au target with an energy of approximately 145 MeV/nucleon. An array of high-purity germanium cluster detectors and large-volume BaF2 scintillator detectors were employed for γ -ray spectroscopy at the secondary target position. The Lund-York-Cologne Calorimeter was used to track the outgoing ions and to identify the nuclear reaction channels. For the two lowest energy excited states of 33Ar the reduced transition strengths have been determined. With these first results the Tz=-3 /2 nucleus 33Ar is now, together with 21Na (Tz=-1 /2 ), the only neutron-deficient odd-A s d shell nucleus in which experimental transition strengths are available. The experimental values are compared to results of shell-model calculations which describe simultaneously mirror-energy differences and transition-strength values of mirror pairs in the s d shell in a consistent way.

  7. Detailed modeling of the atmospheric degradation mechanism of very-short lived brominated species

    NASA Astrophysics Data System (ADS)

    Krysztofiak, G.; Catoire, V.; Poulet, G.; Marécal, V.; Pirre, M.; Louis, F.; Canneaux, S.; Josse, B.

    2012-11-01

    Detailed chemical reaction schemes for the atmospheric degradations of the very short-lived species (VSLS) bromoform (CHBr3) and dibromomethane (CH2Br2) have been established. These degradation schemes have been implemented in the meteorological/tracer transport model CATT-BRAMS used in the present case as pseudo one-dimensional model with chemistry of CH4, CO, HOx, NOx, NOy and Ox. They include the main possible reactions of the intermediate brominated peroxy radicals RO2 (with R = CH2Br, CHBr2 and CBr3) for which the most likely reaction pathways with HO2 have been found using ab initio computational calculations. The full degradation schemes have been run for two well-defined realistic scenarios, “clean” atmosphere and “moderately” NOy-polluted atmosphere, as representative of a tropical coastal region where these VSLS natural emissions are expected to be important. The Henry's law constants of the brominated organics products have been estimated by using the Bond Contribution Method (BCM; Meylan and Howard, 1991) or the Molecular Connectivity Index (MCI; Nirmalakhandan and Speece, 1988). Using these constants, the least soluble species formed from the VSLS degradation are found to be CBr2O, CHBrO, CBr3O2NO2, CHBr2O2NO2, BrO, BrONO2 and HOBr, which leads those to be potentially transported into the tropical tropopause layer (TTL) in case of deep convection and contribute to stratospheric bromine additionally to the original substances. For bromoform and dibromomethane degradation, the moderate NOy pollution increases the production of the least soluble species and thus approximately doubles the bromine quantity potentially able to reach the TTL (from 22.5% to 43% for CHBr3 and from 8.8% to 20.2% for CH2Br2). The influence of the reactions of the RO2 radicals with HO2, CH3O2 and NO2 on the nature and abundance of the stable intermediate and end-products has been tested for CHBr3 degradation. As a result, the reactions of the RO2 radicals with NO2 have no

  8. Global properties of nuclei from {sup 100}Sn to {sup 132}Sn

    SciTech Connect

    Isakov, V. I.

    2013-07-15

    The paper presents the results of both microscopical and semi-empirical calculations of single-particle characteristics, nuclear binding, and one-nucleon separation energies of nuclei, as well as their root-mean-square radii, energy levels and transition rates in the long chain of Sn isotopes. We consider nuclei from the extremely neutron-deficient {sup 100}Sn up to neutron excess {sup 136}Sn, where the experimental information is available by now. The comprehensive comparison with the experimental data is carried out.

  9. Photodissociation experiments for p-process nuclei

    NASA Astrophysics Data System (ADS)

    Wagner, A.; Erhard, M.; Grosse, E.; Junghans, A. R.; Klug, J.; Kosev, K.; Nair, C.; Nankov, N.; Rusev, G.; Schilling, K. D.; Schwengner, R.

    2006-04-01

    The near-threshold photodissociation of nuclides received an increased attention in recent years due to its relevance for heavy element production in astrophysical scenarios. Therefore, a research program has been started to study photodissociation reactions using energetic bremsstrahlung from the new ELBE electron linear accelerator. Special emphasis was devoted to the neutron deficient nuclei with A≈100 which may have been produced in cosmic high-temperature regions by (γ,n), (γ,p), or (γ, α)-reactions. First data were obtained for the astrophysically important target nucleus 92Mo by observing the radioactive decay of the nuclides produced by bremsstrahlung irradiation at end-point energies between 11.8 and 14.0 MeV. The results are compared to recent statistical-model calculations.

  10. Direct mass measurements of short-lived A=2Z-1 nuclides (63)Ge, (65)As, (67)Se, and (71)Kr and their impact on nucleosynthesis in the rp process.

    PubMed

    Tu, X L; Xu, H S; Wang, M; Zhang, Y H; Litvinov, Yu A; Sun, Y; Schatz, H; Zhou, X H; Yuan, Y J; Xia, J W; Audi, G; Blaum, K; Du, C M; Geng, P; Hu, Z G; Huang, W X; Jin, S L; Liu, L X; Liu, Y; Ma, X; Mao, R S; Mei, B; Shuai, P; Sun, Z Y; Suzuki, H; Tang, S W; Wang, J S; Wang, S T; Xiao, G Q; Xu, X; Yamaguchi, T; Yamaguchi, Y; Yan, X L; Yang, J C; Ye, R P; Zang, Y D; Zhao, H W; Zhao, T C; Zhang, X Y; Zhan, W L

    2011-03-18

    Mass excesses of short-lived A=2Z-1 nuclei (63)Ge, (65)As, (67)Se, and (71)Kr have been directly measured to be -46,921(37), -46,937(85), -46,580(67), and -46,320(141)  keV, respectively. The deduced proton separation energy of -90(85)  keV for (65)As shows that this nucleus is only slightly proton unbound. X-ray burst model calculations with the new mass excess of (65)As suggest that the majority of the reaction flow passes through (64)Ge via proton capture, indicating that (64)Ge is not a significant rp-process waiting point. PMID:21469858

  11. Bayes’ Theorem and Early Solar Short-lived Radionuclides: The Case for an Unexceptional Origin for the Solar System

    NASA Astrophysics Data System (ADS)

    Young, Edward D.

    2016-08-01

    The presence of excesses of short-lived radionuclides in the early solar system evidenced in meteorites has been taken as testament to close encounters with exotic nucleosynthetic sources, including supernovae or AGB stars. An analysis of the likelihoods associated with different sources of these extinct nuclides in the early solar system indicates that, rather than being exotic, their abundances were typical of star-forming regions like those observed today in the Galaxy. The radiochemistry of the early solar system is therefore unexceptional, being the consequence of extensive averaging of solids from molecular clouds.

  12. Impact of preindustrial to present-day changes in short-lived pollutant emissions on atmospheric composition and climate forcing

    NASA Astrophysics Data System (ADS)

    Naik, Vaishali; Horowitz, Larry W.; Fiore, Arlene M.; Ginoux, Paul; Mao, Jingqiu; Aghedo, Adetutu M.; Levy, Hiram

    2013-07-01

    We describe and evaluate atmospheric chemistry in the newly developed Geophysical Fluid Dynamics Laboratory chemistry-climate model (GFDL AM3) and apply it to investigate the net impact of preindustrial (PI) to present (PD) changes in short-lived pollutant emissions (ozone precursors, sulfur dioxide, and carbonaceous aerosols) and methane concentration on atmospheric composition and climate forcing. The inclusion of online troposphere-stratosphere interactions, gas-aerosol chemistry, and aerosol-cloud interactions (including direct and indirect aerosol radiative effects) in AM3 enables a more complete representation of interactions among short-lived species, and thus their net climate impact, than was considered in previous climate assessments. The base AM3 simulation, driven with observed sea surface temperature (SST) and sea ice cover (SIC) over the period 1981-2007, generally reproduces the observed mean magnitude, spatial distribution, and seasonal cycle of tropospheric ozone and carbon monoxide. The global mean aerosol optical depth in our base simulation is within 5% of satellite measurements over the 1982-2006 time period. We conduct a pair of simulations in which only the short-lived pollutant emissions and methane concentrations are changed from PI (1860) to PD (2000) levels (i.e., SST, SIC, greenhouse gases, and ozone-depleting substances are held at PD levels). From the PI to PD, we find that changes in short-lived pollutant emissions and methane have caused the tropospheric ozone burden to increase by 39% and the global burdens of sulfate, black carbon, and organic carbon to increase by factors of 3, 2.4, and 1.4, respectively. Tropospheric hydroxyl concentration decreases by 7%, showing that increases in OH sinks (methane, carbon monoxide, nonmethane volatile organic compounds, and sulfur dioxide) dominate over sources (ozone and nitrogen oxides) in the model. Combined changes in tropospheric ozone and aerosols cause a net negative top

  13. Age-dependent inhalation doses to members of the public from indoor short-lived radon progeny.

    PubMed

    Brudecki, K; Li, W B; Meisenberg, O; Tschiersch, J; Hoeschen, C; Oeh, U

    2014-08-01

    The main contribution of radiation dose to the human lungs from natural exposure originates from short-lived radon progeny. In the present work, the inhalation doses from indoor short-lived radon progeny, i.e., (218)Po, (214)Pb, (214)Bi, and (214)Po, to different age groups of members of the public were calculated. In the calculations, the age-dependent systemic biokinetic models of polonium, bismuth, and lead published by the International Commission on Radiological Protection (ICRP) were adopted. In addition, the ICRP human respiratory tract and gastrointestinal tract models were applied to determine the deposition fractions in different regions of the lungs during inhalation and exhalation, and the absorption fractions of radon progeny in the alimentary tract. Based on the calculated contribution of each progeny to equivalent dose and effective dose, the dose conversion factor was estimated, taking into account the unattached fraction of aerosols, attached aerosols in the nucleation, accumulation and coarse modes, and the potential alpha energy concentration fraction in indoor air. It turned out that for each progeny, the equivalent doses to extrathoracic airways and the lungs are greater than those to other organs. The contribution of (214)Po to effective dose is much smaller compared to that of the other short-lived radon progeny and can thus be neglected in the dose assessment. In fact, 90 % of the effective dose from short-lived radon progeny arises from (214)Pb and (214)Bi, while the rest is from (218)Po. The dose conversion factors obtained in the present study are 17 and 18 mSv per working level month (WLM) for adult female and male, respectively. This compares to values ranging from 6 to 20 mSv WLM(-1) calculated by other investigators. The dose coefficients of each radon progeny calculated in the present study can be used to estimate the radiation doses for the population, especially for small children and women, in specific regions of the world

  14. Production of Short-lived Radionuclides by Protons and Neutrons in Fe and Ni Targets: Cross Sections Needed for Cosmic Ray Studies

    NASA Technical Reports Server (NTRS)

    Sisterson, J. M.; Vincent, J.; Jones, D. T. L.; Binns, P. J.; Langen, K.; Schroeder, I.; Buthelezi, Z.; Brooks, F. D.; Buffler, A.; Allie, M. S.

    2000-01-01

    New neutron and proton cross sections for short-lived radionuclides produced in Fe and Ni are presented. These cross sections are essential to understand cosmic ray interactions with meteorites and the lunar surface.

  15. Studies of images of short-lived events using ERTS data. [forest fires, oil spills, vegetation damage, volcanoes, storm ridges, earthquakes, and floods

    NASA Technical Reports Server (NTRS)

    Deutschman, W. A. (Principal Investigator)

    1973-01-01

    The author has identified the following significant results. Detection of short-lived events has continued. Forest fires, oil spills, vegetation damage, volcanoes, storm ridges, earthquakes, and floods have been detected and analyzed.

  16. A generalized method for characterization of 235U and 239Pu content using short-lived fission product gamma spectroscopy

    DOE PAGESBeta

    Knowles, Justin R.; Skutnik, Steven E.; Glasgow, David C.; Kapsimalis, Roger J.

    2016-06-23

    Rapid non-destructive assay methods for trace fissile material analysis are needed in both nuclear forensics and safeguards communities. To address these needs, research at the High Flux Isotope Reactor Neutron Activation Analysis laboratory has developed a generalized non-destructive assay method to characterize materials containing fissile isotopes. This method relies on gamma-ray emissions from short-lived fission products and capitalizes off of differences in fission product yields to identify fissile compositions of trace material samples. Although prior work has explored the use of short-lived fission product gamma-ray measurements, the proposed method is the first to provide a holistic characterization of isotopic identification,more » mass ratios, and absolute mass determination. Successful single fissile isotope mass recoveries of less than 6% error have been conducted on standards of 235U and 239Pu as low as 12 nanograms in less than 10 minutes. Additionally, mixtures of fissile isotope standards containing 235U and 239Pu have been characterized as low as 229 nanograms of fissile mass with less than 12% error. The generalizability of this method is illustrated by evaluating different fissile isotopes, mixtures of fissile isotopes, and two different irradiation positions in the reactor. Furthermore, it is anticipated that this method will be expanded to characterize additional fissile nuclides, utilize various irradiation sources, and account for increasingly complex sample matrices.« less

  17. Alterations in oxidative, inflammatory and apoptotic events in short-lived and long-lived mice testes

    PubMed Central

    Matzkin, María Eugenia; Miquet, Johanna Gabriela; Fang, Yimin; Hill, Cristal Monique; Turyn, Daniel; Calandra, Ricardo Saúl; Bartke, Andrzej; Frungieri, Mónica Beatriz

    2016-01-01

    Aged testes undergo profound histological and morphological alterations leading to a reduced functionality. Here, we investigated whether variations in longevity affect the development of local inflammatory processes, the oxidative state and the occurrence of apoptotic events in the testis. To this aim, well-established mouse models with delayed (growth hormone releasing hormone-knockout and Ames dwarf mice) or accelerated (growth hormone-transgenic mice) aging were used. We hereby show that the testes of short-lived mice show a significant increase in cyclooxygenase 2 expression, PGD2 production, lipid peroxidation, antioxidant enzymes expression, local macrophages and TUNEL-positive germ cells numbers, and the levels of both pro-caspase-3 and cleaved caspase-3. In contrast, although the expression of antioxidant enzymes remained unchanged in testes of long-lived mice, the remainder of the parameters assessed showed a significant reduction. This study provides novel evidence that longevity confers anti-inflammatory, anti-oxidant and anti-apoptotic capacities to the adult testis. Oppositely, short-lived mice suffer testicular inflammatory, oxidative and apoptotic processes. PMID:26805572

  18. Short-lived mammals (shrew, mouse) have a less robust metal-responsive transcription factor than humans and bats.

    PubMed

    Schmidt, Katharina; Steiner, Kurt; Petrov, Boyan; Georgiev, Oleg; Schaffner, Walter

    2016-06-01

    Non-essential "heavy" metals such as cadmium tend to accumulate in an organism and thus are a particular threat for long-lived animals. Here we show that two unrelated, short-lived groups of mammals (rodents and shrews, separated by 100 Mio years of evolution) each have independently acquired mutations in their metal-responsive transcription factor (MTF-1) in a domain relevant for robust transcriptional induction by zinc and cadmium. While key amino acids are mutated in rodents, in shrews an entire exon is skipped. Rodents and especially shrews are unique regarding the alterations of this region. To investigate the biological relevance of these alterations, MTF-1s from the common shrew (Sorex araneus), the mouse, humans and a bat (Myotis blythii), were tested by cotransfection with a reporter gene into cells lacking MTF-1. Whereas shrews only live for 1.5-2.5 years, bats, although living on a very similar insect diet, have a lifespan of several decades. We find that bat MTF-1 is similarly metal-responsive as its human counterpart, while shrew MTF-1 is less responsive, similar to mouse MTF-1. We propose that in comparison to most other mammals, the short-lived shrews and rodents can afford a "lower-quality" system for heavy metal homeostasis and detoxification. PMID:27067444

  19. Sediment Dating With Short-Lived Radioisotopes In Monterey Canyon, California Imply Episodes Of Rapid Deposition And Erosion

    NASA Astrophysics Data System (ADS)

    Lorenson, T. D.; Swarzenski, P. W.; Maier, K. L.; Gwiazda, R.; Paull, C. K.; Sumner, E.; Symons, W. O.

    2015-12-01

    Submarine canyons are a major conduit for terrestrial material to the deep sea. To better constrain the timing and rates in which sediment is transported down-canyon, we collected a series of sediment cores along the axis of Monterey Canyon, and quantified mass accumulation rates using short-lived radio-isotopes. A suite of sediment cores were carefully collected perpendicular to the canyon thalweg in water depths of approximately 300m, 500m, 800m, and 1500m using a remotely operated vehicle (ROV). We choose cores that were between 60m and 75m above the canyon thalweg on canyon side bench features for correlation with moored instrument deployments. The sediment cores reveal a complex stratigraphy that includes copious bioturbation features, sand lenses, subtle erosional surfaces, subtle graded bedding, and abrupt changes sediment texture and color. Downcore excess 210Pb and 137Cs profiles imply episodic deposition and remobilization cycles on the canyon benches. Excess 210Pb activities in cores reach depths of up to 1m, implying very rapid sedimentation. Sedimentation rates vary with water depth, generally with the highest sedimentation rate in closest to land, but vary substantially on adjacent canyon benches. Preliminary results demonstrate that sediment movement within Monterey Canyon is both dynamic and episodic on human time-scales and can be reconstructed used short-lived radio-isotopes.

  20. Overview of the methods for the measurement and interpretation of short-lived radioisotopes and their limits

    NASA Astrophysics Data System (ADS)

    Ghaleb, B.

    2009-01-01

    The daughter products of the uranium and thorium series consist of several radioactive isotopes with half-lives varying from less than a second to 105 years. Combining their half-live with their geochemical behaviour some of these radioisotopes could be used as tracers and/or chronometers of sedimentary processes. For example, thorium isotopes, and to a lesser extent polonium isotopes are characterized by very low solubility and very high affinity for the surface of particles. Consequently, thorium isotopes can be used to document scavenging and adsorption processes. On the other hand, radium isotopes tend to remain in solution and can be used to document diffusion processes. In the following, we present the analytical methods for the measurement and analysis of the most common short-lived isotopes and throughout their utility in studying sedimentary processes will be illustrated by a few examples of applications. These examples will focus essentially on the applications of short lived thorium isotopes (notably 234Th) and the use of 210Pb as chronometer for recent sedimentary accumulation.

  1. Temperature affects longevity and age-related locomotor and cognitive decay in the short-lived fish Nothobranchius furzeri.

    PubMed

    Valenzano, Dario R; Terzibasi, Eva; Cattaneo, Antonino; Domenici, Luciano; Cellerino, Alessandro

    2006-06-01

    Temperature variations are known to modulate aging and life-history traits in poikilotherms as different as worms, flies and fish. In invertebrates, temperature affects lifespan by modulating the slope of age-dependent acceleration in death rate, which is thought to reflect the rate of age-related damage accumulation. Here, we studied the effects of temperature on aging kinetics, aging-related behavioural deficits, and age-associated histological markers of senescence in the short-lived fish Nothobranchius furzeri. This species shows a maximum captive lifespan of only 3 months, which is tied with acceleration in growth and expression of aging biomarkers. These biological peculiarities make it a very convenient animal model for testing the effects of experimental manipulations on life-history traits in vertebrates. Here, we show that (i) lowering temperature from 25 degrees C to 22 degrees C increases both median and maximum lifespan; (ii) life extension is due to reduction in the slope of the age-dependent acceleration in death rate; (iii) lowering temperature from 25 degrees C to 22 degrees C retards the onset of age-related locomotor and learning deficits; and (iv) lowering temperature from 25 degrees C to 22 degrees C reduces the accumulation of the age-related marker lipofuscin. We conclude that lowering water temperature is a simple experimental manipulation which retards the rate of age-related damage accumulation in this short-lived species. PMID:16842500

  2. A GENERALIZED METHOD FOR CHARACTERIZATION OF 235U AND 239PU CONTENT USING SHORT-LIVED FISSION PRODUCT GAMMA SPECTROSCOPY

    SciTech Connect

    Knowles, Justin R; Skutnik, Steven E; Glasgow, David C; Kapsimalis, Roger J

    2016-01-01

    Rapid non-destructive assay methods for trace fissile material analysis are needed in both nuclear forensics and safeguards communities. To address these needs, research at the High Flux Isotope Reactor Neutron Activation Analysis laboratory has developed a generalized non-destructive assay method to characterize materials containing fissile isotopes. This method relies on gamma-ray emissions from short-lived fission products and capitalizes off of differences in fission product yields to identify fissile compositions of trace material samples. Although prior work has explored the use of short-lived fission product gamma-ray measurements, the proposed method is the first to provide a holistic characterization of isotopic identification, mass ratios, and absolute mass determination. Successful single fissile isotope mass recoveries of less than 6% error have been conducted on standards of 235U and 239Pu as low as 12 nanograms in less than 10 minutes. Additionally, mixtures of fissile isotope standards containing 235U and 239Pu have been characterized as low as 229 nanograms of fissile mass with less than 12% error. The generalizability of this method is illustrated by evaluating different fissile isotopes, mixtures of fissile isotopes, and two different irradiation positions in the reactor. It is anticipated that this method will be expanded to characterize additional fissile nuclides, utilize various irradiation sources, and account for increasingly complex sample matrices.

  3. Trace analysis of short-lived iodine-containing volatiles emitted by different types of algae

    NASA Astrophysics Data System (ADS)

    Thorenz, U. R.; Kundel, M.; Huang, R.-J.; Hoffmann, T.

    2012-04-01

    Atmospheric iodine chemistry in the lower troposphere gained more attention in the last decade, because of its role in depleting tropospheric ozone and accelerating the ozone destroying capacity of other halogen species [1]. The iodine oxides formed during this reaction may also undergo further oxidation and form polyoxides which then can act as cloud condensation nuclei [2]. Precursors of both reactions are gaseous molecular iodine (I2) and volatile iodocarbons. Both I2 and iodocarbons are emitted by different kinds of macroalgae, whereby the emission of I2 dominates [3]. Iodocarbons are also released by different kinds of microalgaeand itis assumed that also I2 is released by these algae. Here we present the results of the measurement of iodine containing volatiles emitted by eight different macroalgae found in the intertidal zone and microalgae, two pure cultures and two net samples. To measure I2 emissionfrom macroalgae an on-line time-of-flight aerosol mass spectrometric method was used[4] to determine the emission rates and to investigate temporally resolved emission profiles. The molecular iodine emissions from microalgae were measured using a recently developed denuder sampling technique and GC-MS method [5]. Iodocarbons were preconcentrated on solid adsorbent tubes and measured using thermodesorption-GC-MS. The results of the macroalgae experiments showed that Laminariales were found to be the strongest I2 emitters. Time series of the iodine release of L. digitata and L. hyperborea showed a strong I2 emission when first exposed to air followed by an exponential decline of the release rate. For both species I2 emission bursts were observed. For L. saccharina und F. serratus a more continuous I2 release profile was detected, however, F. serratus released much less I2. For A. nodosum and F. vesiculosus the I2 emission rates were slowly increasing with time (1h-2h) until a more or less stable I2 emission rate was reached. The lowest I2 emission rates were

  4. The analysis of predictability of recent alpha decay formulae and the alpha partial half-lives of some exotic nuclei

    SciTech Connect

    Dasgupta-Schubert, N.; Reyes, M. A.; Tamez, V. A.

    2009-04-20

    Alpha decay is one of the two main decay modes of the heaviest nuclei, (SHE), and constitutes one of the dominant decay modes of highly neutron deficient medium mass nuclei ('exotics'). Thus identifying and characterizing the alpha decay chains form a crucial part of the identification of SHE. We report the extension of the previously developed method for the detailed and systematic investigation of the reliability of the three main extant analytical formulae of alpha decay half-lives: the generalized liquid drop model based formula of Royer et al. (FR), the Sobiczewski modified semi-empirical Viola-Seaborg formula (VSS) and the recent phenomenological formula of Sobiczewski and Parkhomenko (SP)

  5. Identifying and quantifying short-lived fission products from thermal fission of HEU using portable HPGe detectors

    SciTech Connect

    Pierson, Bruce D.; Finn, Erin C.; Friese, Judah I.; Greenwood, Lawrence R.; Kephart, Jeremy D.; Kephart, Rosara F.; Metz, Lori A.

    2013-03-01

    Due to the emerging potential for trafficking of special nuclear material, research programs are investigating current capabilities of commercially available portable gamma ray detection systems. Presented in this paper are the results of three different portable high-purity germanium (HPGe) detectors used to identify short-lived fission products generated from thermal neutron interrogation of small samples of highly enriched uranium. Samples were irradiated at the Washington State University (WSU) Nuclear Radiation Center’s 1MW TRIGA reactor. The three portable, HPGe detectors used were the ORTEC MicroDetective, the ORTEC Detective, and the Canberra Falcon. Canberra’s GENIE-2000 software was used to analyze the spectral data collected from each detector. Ultimately, these three portable detectors were able to identify a large range of fission products showing potential for material discrimination.

  6. Calcium influx through TRP channels induced by short-lived reactive species in plasma-irradiated solution.

    PubMed

    Sasaki, Shota; Kanzaki, Makoto; Kaneko, Toshiro

    2016-01-01

    Non-equilibrium helium atmospheric-pressure plasma (He-APP), which allows for a strong non-equilibrium chemical reaction of O2 and N2 in ambient air, uniquely produces multiple extremely reactive products, such as reactive oxygen species (ROS), in plasma-irradiated solution. We herein show that relatively short-lived unclassified reactive species (i.e., deactivated within approximately 10 min) generated by the He-APP irradiation can trigger physiologically relevant Ca(2+) influx through ruthenium red- and SKF 96365-sensitive Ca(2+)-permeable channel(s), possibly transient receptor potential channel family member(s). Our results provide novel insight into understanding of the interactions between cells and plasmas and the mechanism by which cells detect plasma-induced chemically reactive species, in addition to facilitating development of plasma applications in medicine. PMID:27169489

  7. Corrections for the combined effects of decay and dead time in live-timed counting of short-lived radionuclides.

    PubMed

    Fitzgerald, R

    2016-03-01

    Studies and calibrations of short-lived radionuclides, for example (15)O, are of particular interest in nuclear medicine. Yet counting experiments on such species are vulnerable to an error due to the combined effect of decay and dead time. Separate decay corrections and dead-time corrections do not account for this issue. Usually counting data are decay-corrected to the start time of the count period, or else instead of correcting the count rate, the mid-time of the measurement is used as the reference time. Correction factors are derived for both those methods, considering both extending and non-extending dead time. Series approximations are derived here and the accuracy of those approximations are discussed. PMID:26682893

  8. Prompt gamma activation analysis (PGAA) and short-lived neutron activation analysis (NAA) applied to the characterization of legacy materials

    SciTech Connect

    Firestone, Richard B; English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Leung, Ka-Ngo; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.

    2008-02-13

    Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents.1-3. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity.

  9. Using Atmospheric Dispersion Theory to Inform the Design of a Short-lived Radioactive Particle Release Experiment.

    PubMed

    Rishel, Jeremy P; Keillor, Martin E; Arrigo, Leah M; Baciak, James E; Detwiler, Rebecca S; Kernan, Warnick J; Kirkham, Randy R; Milbrath, Brian D; Seifert, Allen; Seifert, Carolyn E; Smart, John E

    2016-05-01

    Atmospheric dispersion theory can be used to predict ground deposition of particulates downwind of a radionuclide release. This paper uses standard formulations found in Gaussian plume models to inform the design of an experimental release of short-lived radioactive particles into the atmosphere. Specifically, a source depletion algorithm is used to determine the optimum particle size and release height that maximizes the near-field deposition while minimizing both the required source activity and the fraction of activity lost to long-distance transport. The purpose of the release is to provide a realistic deposition pattern that might be observed downwind of a small-scale vent from an underground nuclear explosion. The deposition field will be used, in part, to study several techniques of gamma radiation survey and spectrometry that could be used by an On-Site Inspection team investigating such an event. PMID:27023039

  10. Calcium influx through TRP channels induced by short-lived reactive species in plasma-irradiated solution

    PubMed Central

    Sasaki, Shota; Kanzaki, Makoto; Kaneko, Toshiro

    2016-01-01

    Non-equilibrium helium atmospheric-pressure plasma (He-APP), which allows for a strong non-equilibrium chemical reaction of O2 and N2 in ambient air, uniquely produces multiple extremely reactive products, such as reactive oxygen species (ROS), in plasma-irradiated solution. We herein show that relatively short-lived unclassified reactive species (i.e., deactivated within approximately 10 min) generated by the He-APP irradiation can trigger physiologically relevant Ca2+ influx through ruthenium red- and SKF 96365-sensitive Ca2+-permeable channel(s), possibly transient receptor potential channel family member(s). Our results provide novel insight into understanding of the interactions between cells and plasmas and the mechanism by which cells detect plasma-induced chemically reactive species, in addition to facilitating development of plasma applications in medicine. PMID:27169489

  11. Thyroid cancer in the Marshallese: relative risk of short-lived internal emitters and external radiation exposure

    SciTech Connect

    Lessard, E.T.; Brill, A.B.; Adams, W.H.

    1985-01-01

    In a study of the comparative effects of internal versus external irradiation of the thyroid in young people, we determined that the dose from internal irradiation of the thyroid with short-lived internal emitters produced several times less thyroid cancer than did the same dose of radiation given externally. We determined this finding for a group of 85 Marshall Islands children, who were less than 10 years of age at the time of exposure and who were accidentially exposed to internal and external thyroid radiation at an average level of 1400 rad. The external risk coefficient ranged between 2.5 and 4.9 cancers per million person-rad-years at risk, and thus, from our computations, the internal risk coefficient for the Marshallese children was estimated to range between 1.0 and 1.4 cancers per million person-rad-years at risk. In contrast, for individual more than 10 years of age at the time of exposure, the dose from internal irradiation of the thyroid with short-lived internal emitters produced several times more thyroid cancer than did the same dose of radiation given externally. The external risk coefficients for the older age groups were reported in the literature to be in the range of 1.0 to 3.3 cancers per million person-rad-years-at risk. We computed internal risk coefficients of 3.3 to 8.1 cancers per million person-rad-years at risk for adolescent and adult groups. This higher sensitivity to cancer induction in the exposed adolescents and adults, is different from that seen in other exposed groups. 14 refs., 8 tabs.

  12. Impact of Very Short-live Halogens on Stratospheric Ozone Abundance (and UV radiation) in a Geo-engineered Atmosphere

    NASA Astrophysics Data System (ADS)

    Tilmes, Simone; Kinnison, Doug; Garcia, Rolando; Salawitch, Ross; Lee-Taylor, Julia

    2010-05-01

    In this study we used the Whole Atmosphere Community Climate Model (WACCM) to explore the impact of very short-lived (VSL) bromocarbons on stratospheric ozone abundance and surface UV radiation under the influence of geoengineered aerosols. VSL bromocarbons have by definition a chemical lifetime of less than 0.5 years (WMO, 2006). In contrast to long-lived bromocarbons (e.g., CH3Br plus halons), these VSL bromocarbons have natural sources (e.g., oceanic emissions) and their abundance will therefore not decrease in the future due to international protocols. They are eventually oxidized via reactions with OH and photolysis to form inorganic bromine product gases and get transported into the stratosphere. Observations suggest that VSL bromocarbons add an additional 4-10 pptv volume mixing ratios to the total stratospheric inorganic bromine abundance. Since inorganic bromine is ~60 times more efficient (relative to inorganic chlorine) at catalytic destroying ozone, this additional inorganic bromine loading could significantly affect stratospheric ozone. This is especially true in the Arctic, where the coupled BrO/ClO catalytic ozone loss cycle is as important as the ClO dimer ozone loss cycle. The chemical activation of chlorine is highly dependent on the amount of sulfate aerosol and VSL bromine provides a reaction partner for activated chlorine, resulting in a significant increase of ozone depletion in a geo-engineered aerosol environment in high latitudes. An additional impact of short-lived bromocarbons on the ozone abundance is expected and was not considered in earlier studies.

  13. ON THE INJECTION OF SHORT-LIVED RADIONUCLIDES FROM A SUPERNOVA INTO THE SOLAR NEBULA: CONSTRAINTS FROM THE OXYGEN ISOTOPES

    SciTech Connect

    Liu, Ming-Chang

    2014-02-01

    Injection of short-lived radionuclides from a nearby core-collapse Type II supernova into the already-formed solar protoplanetary disk was proposed to account for the former presence of {sup 26}Al, {sup 41}Ca, and {sup 60}Fe in the early solar system inferred from isotopic analysis of meteoritic samples. One potential corollary of this ''late-injection'' scenario is that the disk's initial (pre-injection) oxygen isotopic composition could be significantly altered, as supernova material that carried the short-lived radionuclides would also deliver oxygen components synthesized in that given star. Therefore, the change in the oxygen isotopic composition of the disk caused by injection could in principle be used to constrain the supernova injection models. Previous studies showed that although supernova oxygen could result in a wide range of shifts in {sup 17}O/{sup 16}O and {sup 18}O/{sup 16}O of the disk, a couple of cases existed where the calculated oxygen changes in the disk would be compatible with the meteoritic and solar wind data. Recently, the initial abundances of {sup 41}Ca and {sup 60}Fe in the solar system were revised to lower values, and the feasibility of supernova injection as a source for the three radionuclides was called into question. In this study, supernova parameters needed for matching {sup 26}Al, {sup 41}Ca, and {sup 60}Fe to their early solar system abundances were reinvestigated and then were used to infer the pre-injection O-isotope composition of the disk. The result suggested that a supernova undergoing mixing fallback might be a viable source for the three radionuclides.

  14. Dicer Regulates the Balance of Short-Lived Effector and Long-Lived Memory CD8 T Cell Lineages.

    PubMed

    Baumann, Florian M; Yuzefpolskiy, Yevgeniy; Sarkar, Surojit; Kalia, Vandana

    2016-01-01

    MicroRNAs constitute a major post-transcriptional mechanism for controlling protein expression, and are emerging as key regulators during T cell development and function. Recent reports of augmented CD8 T cell activation and effector differentiation, and aberrant migratory properties upon ablation of Dicer/miRNAs in naïve cells have established a regulatory role of miRNAs during priming. Whether miRNAs continue to exert similar functions or are dispensable during later stages of CD8 T cell expansion and memory differentiation remains unclear. Here, we report a critical role of Dicer/miRNAs in regulating the balance of long-lived memory and short-lived terminal effector fates during the post-priming stages when CD8 T cells undergo clonal expansion to generate a large cytotoxic T lymphocyte (CTL) pool and subsequently differentiate into a quiescent memory state. Conditional ablation of Dicer/miRNAs in early effector CD8 T cells following optimal activation and expression of granzyme B, using unique dicerfl/fl gzmb-cre mice, led to a strikingly diminished peak effector size relative to wild-type antigen-specific cells in the same infectious milieu. Diminished expansion of Dicer-ablated CD8 T cells was associated with lack of sustained antigen-driven proliferation and reduced accumulation of short-lived effector cells. Additionally, Dicer-ablated CD8 T cells exhibited more pronounced contraction after pathogen clearance and comprised a significantly smaller proportion of the memory pool, despite significantly higher proportions of CD127Hi memory precursors at the effector peak. Combined with previous reports of dynamic changes in miRNA expression as CD8 T cells differentiate from naïve to effector and memory states, these findings support distinct stage-specific roles of miRNA-dependent gene regulation during CD8 T cell differentiation. PMID:27627450

  15. Concentrations of 222Rn, Its Short-Lived Daughters And 212Pb And Their Ratios Under Complex Atmospheric Conditions And Topography

    NASA Astrophysics Data System (ADS)

    Kataoka, Toshio; Yunoki, Eiji; Shimizu, Mitsuo; Mori, Tadashige; Tsukamoto, Osamu; Takahashi, Satoshi; Fudeyasu, Hironori; Ohashi, Yukitaka; Sahashi, Ken; Maitani, Toshihiko; Miyashita, Koh'ichi; Iwata, Toru; Sasaki, Takayuki; Fujikawa, Yoko; Kudo, Akira; Shaw, Roger H.

    Atmospheric activity concentrations of 212Pb and short-lived 222Rndaughters, together with meteorological elements, have been observed continuously atthree sites at Kamisaibara Village in Japan. In addition, atmospheric activity concentrationof 222Rn, equilibrium-equivalent concentration of 222Rn and conditionsof the lower atmosphere were observed for three intensive observation periods at Akawase,one of the three sites in Kamisaibara Village. The equilibrium-equivalent concentration of222Rn is almost the same as the atmospheric activity concentration of short-lived222Rn daughters.The activity concentrations of 212Pb and the short-lived 222Rn daughtersand their ratio were low in the daytime owing to convective mixing, and high at nightowing to the surface-based inversion during periods of no precipitation. Their variationshave several patterns corresponding to the scale of the drainage wind or weak mixing.

  16. Cross Sections Needed for the Interpretation of Long-Lived and Short-Lived Cosmogenic Nuclide Production in Extraterrestrial Materials

    NASA Astrophysics Data System (ADS)

    Sisterson, J. M.; Beverding, A.; Kim, K. J.; Englert, P. A. J.; Jull, A. J. T.; Donahue, D. J.; Cloudt, S.; Castaneda, C.; Vincent, J.; Caffee, M. W.; Osazuwa, C. O.; Reedy, R. C.

    1995-09-01

    Radionuclides produced by cosmic rays in extraterrestrial materials archive information that can be used to determine cosmic-ray fluxes and to study the history of the irradiated object. Long-lived radionuclides give information about the last ~5 Myr; short-lived radionuclides give information about recent events. To calculate the solar cosmic ray (SCR) flux from measured depth profiles for cosmogenic radionuclides produced in lunar rocks, accurate and precise cross section values for the production of these radionuclides from all relevant elements are needed. About 98% of SCR and ~87% of galactic cosmic rays (GCR) falling on extraterrestrial materials are protons. Cross section measurements were made using three proton accelerators to cover the energy range ~20 - 500 MeV. Thin target techniques used in the irradiations minimized the number of protons scattered out of the stack and the neutron production within the stack. After irradiation, the short-lived radionuclides e.g. 22Na, 7Be, 24Na, 54Mn, and 56Co were determined using gamma-ray spectroscopy. 14C, 10Be, and 26Al were determined using Accelerator Mass Spectrometry. Our main objective is to measure the production cross sections of long-lived radionuclides. We have reported new cross section values for making 10Be from O and 14C from O, Mg, Al, Si, Fe, and Ni [1,2]. Using these new results, better estimates for the solar proton flux over several time periods in the past were determined [3]. However, no single value for the SCR flux could explain the measured data from different time periods. Further cross section measurements are being made to verify that the values used in these estimates were accurate. Irradiations designed to give good cross section measurements for long-lived radionuclides also give good cross section measurements for short-lived radionuclides. Results will be presented for proton production cross sections of 22Na from Mg, Al and Si, and 54Mn and 56Co from Fe and Ni; some values at low

  17. Effects of East Asian Short-lived Anthropogenic Air Pollutants on the Northern Hemispheric Air Quality and Climate

    NASA Astrophysics Data System (ADS)

    Liu, J.; Horowitz, L. W.; Lau, N.; Fan, S.; Tao, S.; Mauzerall, D. L.; Levy, H.

    2012-12-01

    Short-lived anthropogenic pollutants (such as ozone and aerosols) not only degrade ambient air quality and influence human health, but also play an important role in scattering/absorbing atmospheric radiation and disturbing regional climate. Due to the rapid industrialization, anthropogenic emissions from East Asia (EA) have increased substantially during the past decades. At the same time, EA has experienced a changing climate in terms of surface temperature and precipitation. In order to understand to what extent that EA short-lived anthropogenic emissions could influence domestic and downwind air quality (e.g. surface O3 and PM2.5), and explore the potential linkage between hemispheric-scale climate perturbation and regional anthropogenic forcing, we simulate global climate and chemical compositions during 1981-2000 based on the coupled general circulation model CM3 for atmosphere (with interactive tropospheric and stratospheric chemistry), oceans, land and sea ice, recently developed at Geophysical Fluid Dynamics Laboratory (GFDL/NOAA). We also conduct a parallel sensitivity simulation which is identical to the base simulation but with all anthropogenic emissions over EA turned off. The difference between the base and sensitivity simulations represents the short-term response of the Northern Hemispheric climate system and atmospheric composition to the perturbation of regional anthropogenic forcing. We find that East Asian short-lived anthropogenic emissions exert significant adverse impacts on local air quality during 1981-2000, accounting for 10-30ppbV daily-averaged O3 over Eastern China in JJA. In particular, EA anthropogenic emissions elevate the summertime daily maximum 8-hour average ozone (MDA8 O3) by 30-40ppbV over the North China Plain, where the typical background MDA8 ozone ranges 30 to 45ppbV. In addition, the surface PM2.5 concentrations peak at the same season and over the same region, with a seasonal mean of 10-30ug/m3, mostly contributed from

  18. Collective degrees of freedom of neutron-rich A≈100 nuclei and the first mass measurement of the short-lived nuclide 100Rb

    NASA Astrophysics Data System (ADS)

    Manea, V.; Atanasov, D.; Beck, D.; Blaum, K.; Borgmann, C.; Cakirli, R. B.; Eronen, T.; George, S.; Herfurth, F.; Herlert, A.; Kowalska, M.; Kreim, S.; Litvinov, Yu. A.; Lunney, D.; Neidherr, D.; Rosenbusch, M.; Schweikhard, L.; Wienholtz, F.; Wolf, R. N.; Zuber, K.

    2013-11-01

    The mass surface in the A˜100 region of the nuclear chart is extended by the measurement of the 98-100Rb isotopes with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The mass of 100Rb is determined for the first time. The studied nuclides mark the known low-Z frontier of the shape transition at N=60. To describe the shape evolution towards the krypton isotopic chain, a theoretical analysis is presented in the framework of the Hartree-Fock-Bogoliubov approach. The importance of the pairing interaction for describing the extent and strength of the region of quadrupole deformation is emphasized. A later transition to large prolate deformation or, alternatively, the predominance of oblate deformation is proposed as explanation for the different behavior of the krypton isotopes. Octupole collectivity is explored as a possible mechanism for the evolution of two-neutron separation energies around N=56.

  19. Plasmacytoid dendritic cells are short-lived: reappraising the influence of migration, genetic factors and activation on estimation of lifespan.

    PubMed

    Zhan, Yifan; Chow, Kevin V; Soo, Priscilla; Xu, Zhen; Brady, Jamie L; Lawlor, Kate E; Masters, Seth L; O'keeffe, Meredith; Shortman, Ken; Zhang, Jian-Guo; Lew, Andrew M

    2016-01-01

    Plasmacytoid dendritic cells (pDCs) play an important role in immunity to certain pathogens and immunopathology in some autoimmune diseases. They are thought to have a longer lifespan than conventional DCs (cDCs), largely based on a slower rate of BrdU labeling by splenic pDCs. Here we demonstrated that pDC expansion and therefore BrdU labeling by pDCs occurs in bone marrow (BM). The rate of labeling was similar between BM pDCs and spleen cDCs. Therefore, slower BrdU labeling of spleen pDCs likely reflects the "migration time" (∼2 days) for BrdU labeled pDCs to traffic to the spleen, not necessarily reflecting longer life span. Tracking the decay of differentiated DCs showed that splenic pDCs and cDCs decayed at a similar rate. We suggest that spleen pDCs have a shorter in vivo lifespan than estimated utilizing some of the previous approaches. Nevertheless, pDC lifespan varies between mouse strains. pDCs from lupus-prone NZB mice survived longer than C57BL/6 pDCs. We also demonstrated that activation either positively or negatively impacted on the survival of pDCs via different cell-death mechanisms. Thus, pDCs are also short-lived. However, the pDC lifespan is regulated by genetic and environmental factors that may have pathological consequence. PMID:27112985

  20. Ozone Destruction in the Upper Troposphere/Lower Stratosphere from Short-Lived Halogens and Climate Impacts

    NASA Astrophysics Data System (ADS)

    Hossaini, Ryan; Chipperfield, Martyn; Montzka, Stephen; Rap, Alex; Dhomse, Sandip; Feng, Wuhu

    2014-05-01

    Halogens released from very short-lived substances (VSLS) can deplete ozone in the upper-troposphere and lower stratosphere where the perturbation can exert a large climate impact. In addition to the known ozone loss from natural biogenic bromine VSLS, such as bromoform (CHBr3), using a global atmospheric model we show that anthropogenic chlorine VSLS such as dichloromethane (CH2Cl2) - not regulated by the Montreal Protocol - also contribute. Although this impact is small compared to bromine VSLS at present, CH2Cl2 has industrial sources and observations show its atmospheric loading is increasing rapidly. We estimate a significant radiative effect of the bromine and chlorine VSLS-driven lower stratospheric ozone destruction of -0.11 Wm-2. The largest impact comes from ozone loss at high latitudes, where column ozone decreases due to VSLS are up to 6%. The trend in anthropogenic chlorine VSLS could cause a significant radiative forcing, especially if augmented by any trend in natural bromine VSLS. We also used the model to study the impact of iodine-containing VSLS such as methyl iodide (CH3I). Of the three halogens iodine has the largest leverage to destroy lower stratospheric ozone, but current limits based on IO observations indicate only a minor impact at present.

  1. Targeted alpha therapy using short-lived alpha-particles and the promise of nanobodies as targeting vehicle

    PubMed Central

    Dekempeneer, Yana; Keyaerts, Marleen; Krasniqi, Ahmet; Puttemans, Janik; Muyldermans, Serge; Lahoutte, Tony; D’huyvetter, Matthias; Devoogdt, Nick

    2016-01-01

    ABSTRACT Introduction: The combination of a targeted biomolecule that specifically defines the target and a radionuclide that delivers a cytotoxic payload offers a specific way to destroy cancer cells. Targeted radionuclide therapy (TRNT) aims to deliver cytotoxic radiation to cancer cells and causes minimal toxicity to surrounding healthy tissues. Recent advances using α-particle radiation emphasizes their potential to generate radiation in a highly localized and toxic manner because of their high level of ionization and short range in tissue. Areas covered: We review the importance of targeted alpha therapy (TAT) and focus on nanobodies as potential beneficial vehicles. In recent years, nanobodies have been evaluated intensively as unique antigen-specific vehicles for molecular imaging and TRNT. Expert opinion: We expect that the efficient targeting capacity and fast clearance of nanobodies offer a high potential for TAT. More particularly, we argue that the nanobodies’ pharmacokinetic properties match perfectly with the interesting decay properties of the short-lived α-particle emitting radionuclides Astatine-211 and Bismuth-213 and offer an interesting treatment option particularly for micrometastatic cancer and residual disease. PMID:27145158

  2. Impact of short-lived non-CO2 mitigation on carbon budgets for stabilizing global warming

    NASA Astrophysics Data System (ADS)

    Rogelj, Joeri; Meinshausen, Malte; Schaeffer, Michiel; Knutti, Reto; Riahi, Keywan

    2015-07-01

    Limiting global warming to any level requires limiting the total amount of CO2 emissions, or staying within a CO2 budget. Here we assess how emissions from short-lived non-CO2 species like methane, hydrofluorocarbons (HFCs), black-carbon, and sulphates influence these CO2 budgets. Our default case, which assumes mitigation in all sectors and of all gases, results in a CO2 budget between 2011-2100 of 340 PgC for a >66% chance of staying below 2°C, consistent with the assessment of the Fifth Assessment Report of the Intergovernmental Panel on Climate Change. Extreme variations of air-pollutant emissions from black-carbon and sulphates influence this budget by about ±5%. In the hypothetical case of no methane or HFCs mitigation—which is unlikely when CO2 is stringently reduced—the budgets would be much smaller (40% or up to 60%, respectively). However, assuming very stringent CH4 mitigation as a sensitivity case, CO2 budgets could be 25% higher. A limit on cumulative CO2 emissions remains critical for temperature targets. Even a 25% higher CO2 budget still means peaking global emissions in the next two decades, and achieving net zero CO2 emissions during the third quarter of the 21st century. The leverage we have to affect the CO2 budget by targeting non-CO2 diminishes strongly along with CO2 mitigation, because these are partly linked through economic and technological factors.

  3. Mood regulation in youth: research findings and clinical approaches to irritability and short-lived episodes of mania like symptoms

    PubMed Central

    Leigh, Eleanor; Smith, Patrick; Milavic, Gordana; Stringaris, Argyris

    2013-01-01

    Purpose of review Mood regulation problems, such as severe chronic irritability or short episodes of mania like symptoms are common, impairing and a topic of intense recent interest to clinicians, researchers and the DSM-5 process. Here we review the most recent findings about these two presentations and discuss approaches to their treatment. Recent findings Longitudinal and genetic findings suggest that chronic irritability should be regarded as a mood problem that is distinct from bipolar disorder. A proportion of children with short (less than 4 days) episodes of mania like symptoms seem to progress to classical (Type I or II) bipolar disorder over time in US clinic samples. In a UK sample, such episodes were independently associated with psychosocial impairment. The evidence base for the treatment of either irritability or short-lived episodes to mania-like symptoms is still small. Clinicians should be cautious with extrapolating treatments from classical bipolar disorder to these mood regulation problems. CBT-based approaches targeting general mood regulation processes may be effective for cases with severe irritability or short episodes of mania like symptoms. Summary There is increasing research evidence for the importance of mood regulation problems in the form of either irritability or short episodes of mania like symptoms in youth. The evidence base for their drug treatment has yet to be developed. CBT-based interventions to modify processes of mood regulation may be a useful and safe intervention for patients with these presentations. PMID:22569307

  4. Constraints on the Origin of Chondrules and CAIs from Short-Lived and Long-Lived Radionuclides

    SciTech Connect

    Kita, N T; Huss, G R; Tachibana, S; Amelin, Y; Nyquist, L E; Hutcheon, I D

    2005-10-24

    The high time resolution Pb-Pb ages and short-lived nuclide based relative ages for CAIs and chondrules are reviewed. The solar system started at 4567.2 {+-} 0.6Ma inferred from the high precision Pb-Pb ages of CAIs. Time scales of CAIs ({le}0.1Myr), chondrules (1-3Myr), and early asteroidal differentiation ({ge}3Myr) inferred from {sup 26}Al relative ages are comparable to the time scale estimated from astronomical observations of young star; proto star, classical T Tauri star and week-lined T Tauri star, respectively. Pb-Pb ages of chondrules also indicate chondrule formation occur within 1-3 Myr after CAIs. Mn-Cr isochron ages of chondrules are similar to or within 2 Myr after CAI formation. Chondrules from different classes of chondrites show the same range of {sup 26}Al ages in spite of their different oxygen isotopes, indicating that chondrule formed in the localized environment. The {sup 26}Al ages of chondrules in each chondrite class show a hint of correlation with their chemical compositions, which implies the process of elemental fractionation during chondrule formation events.

  5. Plasmacytoid dendritic cells are short-lived: reappraising the influence of migration, genetic factors and activation on estimation of lifespan

    PubMed Central

    Zhan, Yifan; Chow, Kevin V.; Soo, Priscilla; Xu, Zhen; Brady, Jamie L.; Lawlor, Kate E.; Masters, Seth L.; O’keeffe, Meredith; Shortman, Ken; Zhang, Jian-Guo; Lew, Andrew M.

    2016-01-01

    Plasmacytoid dendritic cells (pDCs) play an important role in immunity to certain pathogens and immunopathology in some autoimmune diseases. They are thought to have a longer lifespan than conventional DCs (cDCs), largely based on a slower rate of BrdU labeling by splenic pDCs. Here we demonstrated that pDC expansion and therefore BrdU labeling by pDCs occurs in bone marrow (BM). The rate of labeling was similar between BM pDCs and spleen cDCs. Therefore, slower BrdU labeling of spleen pDCs likely reflects the “migration time” (∼2 days) for BrdU labeled pDCs to traffic to the spleen, not necessarily reflecting longer life span. Tracking the decay of differentiated DCs showed that splenic pDCs and cDCs decayed at a similar rate. We suggest that spleen pDCs have a shorter in vivo lifespan than estimated utilizing some of the previous approaches. Nevertheless, pDC lifespan varies between mouse strains. pDCs from lupus-prone NZB mice survived longer than C57BL/6 pDCs. We also demonstrated that activation either positively or negatively impacted on the survival of pDCs via different cell-death mechanisms. Thus, pDCs are also short-lived. However, the pDC lifespan is regulated by genetic and environmental factors that may have pathological consequence. PMID:27112985

  6. Solar Cosmic-ray Interaction with Protoplanetary Disks: Production of Short-lived Radionuclides and Amorphization of Crystalline Material

    NASA Astrophysics Data System (ADS)

    Trappitsch, R.; Ciesla, F. J.

    2015-05-01

    Solar cosmic-ray (SCR) interactions with a protoplanetary disk have been invoked to explain several observations of primitive planetary materials. In our own Solar System, the presence of short-lived radionuclides (SLRs) in the oldest materials has been attributed to spallation reactions induced in phases that were irradiated by energetic particles in the solar nebula. Furthermore, observations of other protoplanetary disks show a mixture of crystalline and amorphous grains, though no correlation between grain crystallinity and disk or stellar properties have been identified. As most models for the origin of crystalline grains would predict such correlations, it was suggested that amorphization by stellar cosmic-rays may be masking or erasing such correlations. Here we quantitatively investigate these possibilities by modeling the interaction of energetic particles emitted by a young star with the surrounding protoplanetary disk. We do this by tracing the energy evolution of SCRs emitted from the young star through the disk and model the amount of time that dust grains would spend in regions where they would be exposed to these particles. We find that this irradiation scenario cannot explain the total SLR content of the solar nebula; however, this scenario could play a role in the amorphization of crystalline material at different locations or epochs of the disk over the course of its evolution.

  7. Estimating surface fluxes of very short-lived halogens from aircraft measurements over the tropical Western Pacific

    NASA Astrophysics Data System (ADS)

    Feng, Liang; Palmer, Paul I.; Butler, Robyn; Harris, Neil; Carpenter, Lucy; Andrews, Steve; Atlas, Elliot; Pan, Laura; Salawitch, Ross; Donets, Valeria; Schauffler, Sue

    2016-04-01

    We use an inverse model approach to quantitatively understand the ocean flux and atmospheric transport of very short-lived halogenated species (VSLS) measured during the coordinated NERC CAST and NCAR CONTRAST aircraft campaigns over the Western Pacific during January/February 2014. To achieve this we have developed a nested GEOS-Chem chemistry transport model simulation of bromoform (CHBr3) and dibromomethane (CH2Br2), which has a spatial resolution of 0.25° (latitude) × 0.3125° (longitude) over the tropical Western Pacific region, and fed by boundary conditions from a coarser version of the model. We use archived 3-hourly 3-D fields of OH and j-values for CHBr3 photolysis, allowing us to linearly decompose these gases into tagged contributions from different geographical regions. Using these tagged tracers, we are able to use the maximum a posteriori probability (MAP) approach to estimate the VSLS sources by fitting the model to observations. We find that the resulting VSLS fluxes are significantly different from some previous studies. To interpret the results, we describe several observation system simulation experiments to understand the sensitivity of these flux estimates to observation errors as well as to the uncertainty in the boundary condition imposed around the nested grid.

  8. Mesenchymal stem cells are short-lived and do not migrate beyond the lungs after intravenous infusion

    PubMed Central

    Eggenhofer, E.; Benseler, V.; Kroemer, A.; Popp, F. C.; Geissler, E. K.; Schlitt, H. J.; Baan, C. C.; Dahlke, M. H.; Hoogduijn, M. J.

    2012-01-01

    Mesenchymal stem cells (MSC) are under investigation as a therapy for a variety of disorders. Although animal models show long term regenerative and immunomodulatory effects of MSC, the fate of MSC after infusion remains to be elucidated. In the present study the localization and viability of MSC was examined by isolation and re-culture of intravenously infused MSC. C57BL/6 MSC (500,000) constitutively expressing DsRed-fluorescent protein and radioactively labeled with Cr-51 were infused via the tail vein in wild-type C57BL/6 mice. After 5 min, 1, 24, or 72 h, mice were sacrificed and blood, lungs, liver, spleen, kidneys, and bone marrow removed. One hour after MSC infusion the majority of Cr-51 was found in the lungs, whereas after 24 h Cr-51 was mainly found in the liver. Tissue cultures demonstrated that viable donor MSC were present in the lungs up to 24 h after infusion, after which they disappeared. No viable MSC were found in the other organs examined at any time. The induction of ischemia-reperfusion injury in the liver did not trigger the migration of viable MSC to the liver. These results demonstrate that MSC are short-lived after i.v. infusion and that viable MSC do not pass the lungs. Cell debris may be transported to the liver. Long term immunomodulatory and regenerative effects of infused MSC must therefore be mediated via other cell types. PMID:23056000

  9. Impact of very short-lived halogens on stratospheric ozone abundance and UV radiation in a geo-engineered atmosphere

    NASA Astrophysics Data System (ADS)

    Tilmes, S.; Kinnison, D. E.; Garcia, R. R.; Salawitch, R.; Canty, T.; Lee-Taylor, J.; Madronich, S.; Chance, K.

    2012-08-01

    The impact of very short-lived (VSL) halogenated source species on the ozone layer and surface erythemal ultraviolet radiation (UVERY) is investigated in the context of geo-engineering of climate by stratospheric sulfur injection. For a projected 2040 model atmosphere, consideration of VSL halogens at their upper limit results in lower ozone columns and higher UVERY due to geo-engineering for nearly all seasons and latitudes, with UVERY rising by 12% and 6% in southern and northern high latitudes, respectively. When VSL halogen sources are neglected, future UVERY increases due to declines in ozone column are nearly balanced by reductions of UVERY due to scattering by the higher stratospheric aerosol burden in mid-latitudes. Consideration of VSL sources at their upper limit tips the balance, resulting in annual average increases in UVERY of up to 5% in mid and high latitudes. Therefore, VSL halogens should be considered in models that assess the impact of stratospheric sulfur injections on the ozone layer.

  10. Impact of very short-lived halogens on stratospheric ozone abundance and UV radiation in a geo-engineered atmosphere

    NASA Astrophysics Data System (ADS)

    Tilmes, S.; Kinnison, D. E.; Garcia, R. R.; Salawitch, R.; Canty, T.; Lee-Taylor, J.; Madronich, S.; Chance, K.

    2012-11-01

    The impact of very short-lived (VSL) halogenated source species on the ozone layer and surface erythemal ultraviolet radiation (UVERY) is investigated in the context of geo-engineering of climate by stratospheric sulfur injection. For a projected 2040 model atmosphere, consideration of VSL halogens at their upper limit results in lower ozone columns and higher UVERY due to geo-engineering for nearly all seasons and latitudes, with UVERY rising by 12% and 6% in southern and northern high latitudes, respectively. When VSL halogen sources are neglected, future UVERY increases due to declines in ozone column are nearly balanced by reductions of UVERY due to scattering by the higher stratospheric aerosol burden in mid-latitudes. Consideration of VSL sources at their upper limit tips the balance, resulting in annual average increases in UVERY of up to 5% in mid and high latitudes. Therefore, VSL halogens should be considered in models that assess the impact of stratospheric sulfur injections on the ozone layer.

  11. Impact of Very Short-lived Halogens on Stratospheric Ozone Abundance and UV radiation in a Geo-engineered Atmosphere

    NASA Astrophysics Data System (ADS)

    Tilmes, S.; Kinnison, D. E.; Garcia, R. R.; Salawitch, R. J.; Canty, T. P.; Lee-Taylor, J.; Madronich, S.; Chance, K.

    2012-12-01

    The impact of BrO from very short-lived (VSL) source species on stratospheric ozone is investigated for a hypothetical geo-engineered atmosphere in 2040, assuming the injection of sulfuric acid aerosols. An estimated amount of stratospheric halogens from VSL sources based on satellite observations, model results and previous studies, result in lower column ozone for nearly all seasons and nearly all latitudes, and up to 4% in summer mid- and high latitudes. Considering an upper limit of VSL sources, the annual increase in surface erythemal UV radiation (UV_ERY) due to the decrease in ozone as a result of geo-engineering is 12% and 6% in southern and northern high latitudes, respectively. The increase of UV_ERY due to a reduction of ozone for low and mid latitudes is balanced by the reduction of UV_ERY due to aerosol scattering, if VSL halogen sources are not considered. However, VSL halogens results in additional ozone depletion and in an increase of UV_ERY of up to 5% in spring and fall in mid- and high latitudes as a result of geo-engineering. This study demonstrates that VSL halogens should be considered in models that assess the impact of stratospheric sulfur injections on the ozone layer.

  12. Shell Model Based Reaction Rates for rp-PROCESS Nuclei in the Mass Range A=44-63

    NASA Astrophysics Data System (ADS)

    Fisker, J. L.; Barnard, V.; Görres, J.; Langanke, K.; Martínez-Pinedo, G.; Wiescher, M. C.

    2001-11-01

    We have used large-scale shell-model diagonalization calculations to determine the level spectra, proton spectroscopic factors, and electromagnetic transition probabilities for proton rich nuclei in the mass range A=44-63. Based on these results and the available experimental data, we calculated the resonances for proton capture reactions on neutron deficient nuclei in this mass range. We also calculated the direct capture processes on these nuclei in the framework of a Woods-Saxon potential model. Taking into account both resonant and direct contributions, we determined the ground-state proton capture reaction rates for these nuclei under hot hydrogen burning conditions for temperatures between 108 and 1010 K. The calculated compound-nucleus level properties and the reaction rates are presented here; the rates are also available in computer-readable format from the authors.

  13. Intruder states and the onset of deformation in the neutron-deficient even-even polonium isotopes

    SciTech Connect

    The ISOLDE Collaboration

    1995-12-01

    Alpha- and beta-decay studies of mass-separated Rn and At nuclei reveal the existence of a low-lying 0{sup +} state in {sup 196,198,200,202}Po. The excited 0{sup +} states are interpreted as proton-pair excitations across the {ital Z}=82 shell gap leading to a deformed state, coexisting with the spherical ground state. It is shown that with decreasing neutron number the deformed configuration intrudes to lower excitation energy, increasingly mixing into the ground state. {copyright} {ital 1995 The American Physical Society.}

  14. The short-lived (<2 minutes) acceleration of protons to >13 GeV in association with solar flares.

    NASA Astrophysics Data System (ADS)

    McCracken, Ken; Shea, Margaret Ann; Smart, Don

    2016-04-01

    release) mechanism must then decrease greatly in efficiency abruptly ~3 minutes after it started. We note that this is not a unique example; the >10GeV particle pulse in the GLE of 20 January 2005 persisted for only 3 minutes; and a >4.5 GeV pulse at the commencement of the GLE of 7 December, 1982, only lasted one minute. We conclude with a comparison between these observations and the predictions of several proposed acceleration models. We conclude that these short-lived bursts of highly relativistic cosmic rays have been accelerated in the reconnection regions associated with large solar flares. In the greater majority of cases, the short-lived, high energy cosmic ray pulse at the commencement of a GLE is followed by a slowly rising component accelerated in the CME generated shock.

  15. Integrated Assessment on Effects of Short-Lived Climate Pollutants (SLCPs) in Asia based on Numerical Models

    NASA Astrophysics Data System (ADS)

    Takemura, T.; Sudo, K.; Ueda, K.; Masutomi, Y.; Watanabe, S.; Nakata, M.; Takahashi, H. G.; Goto, D.

    2015-12-01

    Air pollution over the Asian region is a serious social problem. For example, activities of the Climate and Clean Air Coalition (CCAC) under the UNFCCC focus on raising awareness and improving scientific understanding of short-lived climate pollutant (SLCP) impacts and mitigation strategies. Our Japanese research project is searching an optimum reduction path of SLCPs considering climate change, health impacts, and agricultural damages. For this purpose, we use aerosol and chemistry models, SPRINTARS and CHASER, respectively, which have been developed by our group, coupled with a general circulation model, MIROC. In the phase 1 of this project, changes in concentrations and radiative forcing of each major SLCPs originating from China, east Asia, southeast Asia, and south Asia in the last 30 years are estimated with the models. Transient simulations along the new emission scenario, SSPs (Shared Socio-economic Pathways) are executed using the MIROC-SPRINTARS/CHASER with ocean circulation in the phase 2 to analyze full feedbacks including hydrological cycle affected by SLCPs. These simulated results will be utilized to estimate health and agricultural impacts of SLCPs. In this presentation, we discuss the optimum reduction path of SLCPs taking both mitigation of global warming and air pollution into consideration. Acknowledgements: Simulations in this study were executed with the supercomputer system of the National Institute for Environmental Studies, Japan. This study is partly supported by the Environment Research and Technology Development Fund (S-12-3) of the Ministry of the Environment, Japan and JSPS KAKENHI Grant Number 15H01728 and 15K12190.

  16. Adult neurogenesis in the short-lived teleost Nothobranchius furzeri: localization of neurogenic niches, molecular characterization and effects of aging

    PubMed Central

    Tozzini, Eva Terzibasi; Baumgart, Mario; Battistoni, Giorgia; Cellerino, Alessandro

    2012-01-01

    We studied adult neurogenesis in the short-lived annual fish Nothobranchius furzeri and quantified the effects of aging on the mitotic activity of the neuronal progenitors and the expression of glial fibrillary acid protein (GFAP) in the radial glia. The distribution of neurogenic niches is substantially similar to that of zebrafish and adult stem cells generate neurons, which persist in the adult brain. As opposed to zebrafish, however, the N. furzeri genome contains a doublecortin (DCX) gene. Doublecortin is transiently expressed by newly generated neurons in the telencephalon and optic tectum (OT). We also analyzed the expression of the microRNA miR-9 and miR-124 and found that they have complementary expression domains: miR-9 is expressed in the neurogenic niches of the telencephalon and the radial glia of the OT, while miR-124 is expressed in differentiated neurons. The main finding of this paper is the demonstration of an age-dependent decay in adult neurogenesis. Using unbiased stereological estimates of cell numbers, we detected an almost fivefold decrease in the number of mitotically active cells in the OT between young and old age. This reduced mitotic activity is paralleled by a reduction in DCX labeling. Finally, we detected a dramatic up-regulation of GFAP in the radial glia of the aged brain. This up-regulation is not paralleled by a similar up-regulation of S100B and Musashi-1, two other markers of the radial glia. In summary, the brain of N. furzeri replicates two typical hallmarks of mammalian aging: gliosis and reduced adult neurogenesis. PMID:22171971

  17. Dealing with uncertainty: Response-resilient climate change mitigation polices for long-lived and short-lived climate pollutants

    NASA Astrophysics Data System (ADS)

    Millar, R.; Boneham, J.; Hepburn, C.; Allen, M. R.

    2015-12-01

    Climate change solutions are subject to many inherent uncertainties. One of the most important is the uncertainty over the magnitude of the physical response of the climate system to external forcing. The risk of extremely large responses to forcing, so called "fat-tail" outcomes, cannot be ruled out from the latest science and offer profound challenges when creating policies that aim to meet a specific target of global temperature change. This study offers examples of how mitigation policies can be made resilient to this uncertainty in the physical climate response via indexing policies against an attributable anthropogenic warming index (the magnitude of the observed global mean warming that is can be traced to human activities), the AWI, instead of against time directly. We show that indexing policy measures that influence the total stock of carbon in the atmosphere (such as the fraction of extracted carbon sequestered) against the AWI can largely eliminate the risk of missing the specified warming goal due to unexpectedly large climate responses as well as the risk of costly over-mitigation if the physical response turned out to be lower than expected. We offer further examples of how this methodology can be expanded to include short-lived climate pollutants as well as long-lived carbon dioxide. Indexing policies against the AWI can have important consequences for the actions of governments acting to design national climate mitigation policies as well as private sector investors looking to incentivise the transition to a climate-stable economy. We conclude with some thoughts on how these indexes can help focus attention on the long-term perspective that is consistent with the conclusions of the latest climate science on what is required to ultimately stabilise the global climate system.

  18. How sensitive is the recovery of stratospheric ozone to changes in concentrations of very short-lived bromocarbons?

    NASA Astrophysics Data System (ADS)

    Yang, X.; Abraham, N. L.; Archibald, A. T.; Braesicke, P.; Keeble, J.; Telford, P. J.; Warwick, N. J.; Pyle, J. A.

    2014-10-01

    Naturally produced very short-lived substances (VSLS) account for almost a quarter of the current stratospheric inorganic bromine, Bry. Following VSLS oxidation, bromine radicals (Br and BrO) can catalytically destroy ozone. The extent to which possible increases in surface emissions or transport of these VSLS bromocarbons to the stratosphere could counteract the effect of halogen reductions under the Montreal Protocol is an important policy question. Here, by using a chemistry-climate model, UM-UKCA, we investigate the impact of a hypothetical doubling (an increase of 5 ppt Bry) of VSLS bromocarbons on ozone and how the resulting ozone changes depend on the background concentrations of chlorine and bromine. Our model experiments indicate that for the 5 ppt increase in Bry from VSLS, the ozone decrease in the lowermost stratosphere of the Southern Hemisphere (SH) may reach up to 10% in the annual mean; the ozone decrease in the Northern Hemisphere (NH) is smaller (4-6%). The largest impact on the ozone column is found in the Antarctic spring. There is a significantly larger ozone decrease following the doubling of the VSLS burden under a high stratospheric chlorine background than under a low chlorine background, indicating the importance of the inter-halogen reactions. For example, the decline in the high-latitude, lower-stratospheric ozone concentration as a function of Bry is higher by about 30-40% when stratospheric Cly is ~ 3 ppb (present day), compared with Cly of ~ 0.8 ppb (a pre-industrial or projected future situation). Bromine will play an important role in the future ozone layer. However, even if bromine levels from natural VSLS were to increase significantly later this century, changes in the concentration of ozone will likely be dominated by the decrease in anthropogenic chlorine. Our calculation suggests that for a 5 ppt increase in Bry from VSLS, the Antarctic ozone hole recovery date could be delayed by approximately 6-8 years, depending on Cly

  19. How sensitive is the recovery of stratospheric ozone to changes in concentrations of very short lived bromocarbons?

    NASA Astrophysics Data System (ADS)

    Yang, X.; Abraham, N. L.; Archibald, A. T.; Braesicke, P.; Keeble, J.; Telford, P.; Warwick, N. J.; Pyle, J. A.

    2014-04-01

    Naturally produced very short-lived substances (VSLS), like bromocarbons, account for almost a quarter of the current stratospheric inorganic bromine, Bry. Following VSLS oxidation, bromine radicals (Br and BrO) can catalytically destroy ozone. The extent to which possible increases in surface emissions or transport of these VSLS bromocarbons to the stratosphere could counteract the effect of halogen reductions under the Montreal Protocol is an important policy question. Here by using a chemistry-climate model, UM-UKCA, we investigate the impact of a hypothetical increase in VSLS on ozone and how that impact depends on the background concentrations of chlorine and bromine. Our model experiments indicate that for a ~5 ppt increase in Bry from VSLS, the local ozone loss in the lowermost stratosphere of the Southern Hemisphere (SH) may reach up to 10% in the annual mean; the ozone loss in the Northern Hemisphere (NH) is smaller (4-6%). There is more ozone loss following an increase in VSLS burden under a high stratospheric chlorine background than under a low chlorine background indicating the importance of the inter-halogen reactions. For example, the rate of decline of the stratospheric ozone concentration as a function of Bry is higher by about 30-40% when stratospheric Cly is ~3 ppb (present day) compared with Cly of ~0.8 ppb (apre-industrial or projected future situation). Although bromine plays an important role in destroying ozone, inorganic chlorine is the dominant halogen compound. Even if bromine levels from natural VSLS were to increase significantly later this century, changes in the concentration of ozone will be dominated by the recovery of anthropogenic chlorine. Our calculation suggests that for a 5 ppt increase in Bry from VSLS, the Antarctic ozone hole recover date could be delayed by approximately 7 years.

  20. Short-lived halocarbons efficient at influencing climate through ozone loss in the upper troposphere-lower stratosphere

    NASA Astrophysics Data System (ADS)

    Hossaini, Ryan; Chipperfield, Martyn; Montzka, Steven; Rap, Alex; Dhomse, Sandip; Feng, Wuhu

    2015-04-01

    Halogenated very short-lived substances (VSLS) of both natural and anthropogenic origin are a significant source of atmospheric bromine, chlorine and iodine. Due to relatively short atmospheric lifetimes (typically <6 months), VSLS breakdown in the upper troposphere-lower stratosphere (UTLS), where ozone perturbations drive a disproportionately large climate impact compared to other altitudes. Here we present chemical transport model simulations that quantify VSLS-driven ozone loss in the UTLS and infer the climate relevance of these ozone perturbations using a radiative transfer model. Our results indicate that through their impact on UTLS ozone, VSLS are efficient at influencing climate. We calculate a whole atmosphere global mean radiative effect (RE) of -0.20 (-0.16 to -0.23) Wm-2 from natural and anthropogenic VSLS-driven ozone loss, including a tropospheric contribution of -0.12 Wm-2. In the stratosphere, the RE due to ozone loss from natural bromine-containing VSLS (e.g. CHBr3, CH2Br2) is almost half of that from long-lived anthropogenic compounds (e.g. CFCs) and normalized by equivalent chlorine is ~4 times larger. We show that the anthropogenic chlorine-containing VSLS, not regulated by the Montreal Protocol, also contribute to ozone loss in the UTLS and that the atmospheric concentration of dichloromethane (CH2Cl2), the most abundant of these, is increasing rapidly. Finally, we present evidence that VSLS have made a small yet previously unrecognized contribution to the ozone-driven radiative forcing of climate since pre-industrial times of -0.02 (-0.01 to -0.03) Wm-2. Given the climate leverage that VSLS possess, future increases to their emissions, either through continued industrial or altered natural processes, may be important for future climate forcing.

  1. Transport of very short-lived halocarbons from the Indian Ocean to the stratosphere through the Asian monsoon circulation

    NASA Astrophysics Data System (ADS)

    Fiehn, Alina; Hepach, Helmke; Atlas, Elliot; Quack, Birgit; Tegtmeier, Susann; Krüger, Kirstin

    2016-04-01

    Halogenated organic compounds are naturally produced in the ocean and emitted to the atmosphere. The halogenated very short-lived substances (VSLS), such as bromoform, have atmospheric lifetimes of less than half a year. When VSLS reach the stratosphere, they enhance ozone depletion and thus impact the climate. During boreal summer, the Asian monsoon circulation transfers air masses from the Asian troposphere to the global stratosphere. Still, the extent to which VSLS from the Indian Ocean contribute to the stratospheric halogen burden and their exact origin is unclear. Here we show that the monsoon circulation transports VSLS from the Indian Ocean to the stratosphere. During the research cruises SO234-2 and SO235 in July-August 2014 onboard RV SONNE, we measured oceanic and atmospheric concentrations of bromoform (tropical lifetime at 10 km = 17 days), dibromomethane (150 days) and methyl iodide (3.5 days) in the subtropical and tropical West Indian Ocean and calculated their emission strengths. We use the Langrangian transport model FLEXPART driven by ERA-Interim meteorological fields to investigate the transport of oceanic emissions in the atmosphere. We analyze the direct contribution of observed bromoform emissions to the stratospheric halogen budget with forward trajectories. Furthermore, we investigate the connection between the Asian monsoon anticyclone and the oceanic source regions using backward trajectories. The West Indian Ocean is a strong source region of VSLS to the atmosphere and the monsoon transport is fast enough for bromoform to reach the stratosphere. However, the main source regions for the entrainment of oceanic air masses through the Asian monsoon anticyclone are the West Pacific and Bay of Bengal as well as the Arabian Sea. Our findings indicate that changes in emission or circulation in this area due to climate change can directly affect the stratospheric halogen burden and thus the ozone layer.

  2. The effects of short-lived radionuclides and porosity on the early thermo-mechanical evolution of planetesimals

    NASA Astrophysics Data System (ADS)

    Lichtenberg, Tim; Golabek, Gregor J.; Gerya, Taras V.; Meyer, Michael R.

    2016-08-01

    The thermal history and internal structure of chondritic planetesimals, assembled before the giant impact phase of chaotic growth, potentially yield important implications for the final composition and evolution of terrestrial planets. These parameters critically depend on the internal balance of heating versus cooling, which is mostly determined by the presence of short-lived radionuclides (SLRs), such as 26Al and 60Fe, as well as the heat conductivity of the material. The heating by SLRs depends on their initial abundances, the formation time of the planetesimal and its size. It has been argued that the cooling history is determined by the porosity of the granular material, which undergoes dramatic changes via compaction processes and tends to decrease with time. In this study we assess the influence of these parameters on the thermo-mechanical evolution of young planetesimals with both 2D and 3D simulations. Using the code family I2ELVIS/I3ELVIS we have run numerous 2D and 3D numerical finite-difference fluid dynamic models with varying planetesimal radius, formation time and initial porosity. Our results indicate that powdery materials lowered the threshold for melting and convection in planetesimals, depending on the amount of SLRs present. A subset of planetesimals retained a powdery surface layer which lowered the thermal conductivity and hindered cooling. The effect of initial porosity was small, however, compared to those of planetesimal size and formation time, which dominated the thermo-mechanical evolution and were the primary factors for the onset of melting and differentiation. We comment on the implications of this work concerning the structure and evolution of these planetesimals, as well as their behavior as possible building blocks of terrestrial planets.

  3. Identifying emission source regions and transport pathways of very short-lived halogens over the Western Pacific

    NASA Astrophysics Data System (ADS)

    Butler, Robyn; Palmer, Paul; Feng, Liang; Harris, Neil; Carpenter, Lucy; Andrews, Steve; Atlas, Elliot; Salawitch, Ross; Pan, Laura; Donets, Valeria; Schauffler, Sue

    2016-04-01

    Deep, tropical convective systems lead to the rapid transport of very short-lived halogenated substances (VSLS) to the tropical tropopause layer (TTL). They are then subsequently transported to the lower stratosphere and chemically broken down to release the constituent halogens that catalytically destroy ozone. Although the oceans are known to represent the largest VSLS source, the relative contribution of geographical regions through emission and transport is poorly understood. We present a study on the origin and variability of VSLS over the Western Pacific using data collected during the CAST and CONTRAST measurement campaigns, January/February 2014. We have developed a version of the GEOS-Chem atmospheric chemistry transport model that tags emissions of bromoform (CHBr3) and dibromomethane (CH2Br2) from different geographical regions. We focus the source regions on land and (coastal and open) oceanic emissions. We have also developed a similar tagged method to calculate the physical age of air parcels from these source regions to quantify the speed of vertical transport. Using this approach we have quantified relative contributions of source regions and show that open oceanic emission regions are the dominant source of VSLS gases during the measurement campaigns. By looking at variability over the region, we see that this is caused by direct convection of marine emissions over the open ocean leading to increased contribution to CHBr3 and CH2Br2 mixing ratios from this source region. Open oceanic emissions are transported to the TTL within the average atmospheric lifetime of CHBr3, the shorter lived species, whereas emissions from coastal ocean and land source regions have an older physical age at the TTL. The relative contribution from island land masses in the campaign region have no impact over the vertical profile but does impact local mixing ratios.

  4. Automated system for neutron activation analysis determination of short lived isotopes at The DOW Chemical Company's TRIGA research reactor

    NASA Astrophysics Data System (ADS)

    Zieman, J. J.; Rigot, W. L.; Romick, J. D.; Quinn, T. J.; Kocher, C. W.

    1994-12-01

    An automated neutron activation analysis (NAA) system for the determination of short lived isotopes was constructed at The DOW Chemical Company's TRIGA Research Reactor in 1993. The NAA group of the Analytical Sciences Laboratory uses the reactor for thousands of analyses each year and therefore automation is important to achieve and maintain high throughput and precision (productivity). This project is complementary to automation of the long-lived counting facilities (see Romick et al., these Proceedings). Canberra/Nuclear Data Systems DEC-based software and electronics modules and an I/O mounting board are the basic commercial components. A Fortran program on a VAX computer controls I/O via ethernet to an Acquisition Interface Module (AIM). The AIM controls the γ spectrometer modules and is interfaced to a Remote Parallel Interface (RPI) module which controls the pneumatic transfer apparatus with TTL signals to the I/O mounting board. Near-infrared sensors are used to monitor key points in the transfer system. Spectra are acquired by a single HPGe detector mounted on a sliding rail to allow flexible and more reproducible counting geometries than with manual sample handling. The maximum sample size is 8 ml in a heat-sealed two dram vial. The sample vial is nested into a "rabbit" vial for irradiation which can be automatically removed prior to spectrum collection. The system was designed to be used by the reactor operator at the control console without the aid of an additional experimenter. Applications include the determination of selenium and silver in coal and water, fluorine in tetra-fluoro ethylene (TFE) coated membranes, aluminum and titanium in composite materials and trace fluorine in non-chlorinated cleaning solvents. Variable dead time software allows analysis for 77mSe despite high dead times from 16N encountered in samples.

  5. Physical Processing of Cometary Nuclei

    NASA Technical Reports Server (NTRS)

    Weissman, Paul R.; Stern, S. Alan

    1997-01-01

    Cometary nuclei preserve a cosmo-chemical record of conditions and processes in the primordial solar nebula, and possibly even the interstellar medium. However, that record is not perfectly preserved over the age of the solar system due to a variety of physical processes which act to modify cometary surfaces and interiors. Possible structural and/or internal processes include: collisional accretion, disruption, and reassembly during formation; internal heating by long and short-lived radionuclides; amorphous to crystalline phase transitions, and thermal stresses. Identified surface modification processes include: irradiation by galactic cosmic rays, solar protons, UV photons, and the Sun's T Tauri stage mass outflow; heating by passing stars and nearby supernovae; gardening by debris impacts; the accretion of interstellar dust and gas and accompanying erosion by hypervelocity dust impacts and sputtering; and solar heating with accompanying crust formation. These modification processes must be taken into account in both the planning and the interpretation of the results of a Comet Nucleus Sample Return Mission. Sampling of nuclei should be done at as great a depth below the surface crust as technically feasible, and at vents or fissures leading to exposed volatiles at depth. Samples of the expected cometary crust and near-surface layers also need to be returned for analysis to achieve a better understanding of the effects of these physical processes. We stress that comets are still likely less modified dm any other solar system bodies, but the degree of modification can vary greatly from one comet to the next.

  6. Test of the critical point symmetry X(5) in neutron deficient osmium isotopes at A{approx_equal}180

    SciTech Connect

    Dewald, A.; Moeller, O.; Melon, B.; Pissulla, T.; Saha, B.; Heinze, S.; Jolie, J.; Zell, K. O.; Petkov, P.; Bazzacco, D.; Lunardi, S.; Ur, C. A.; Farnea, E.; Menegazzo, R.; De Angelis, G.; Tonev, D.; Napoli, D. R.; Marginean, N.; Martinez, T.; Axiotis, M.

    2006-04-26

    The energy spectra and relative transition rates of 176,178,180Os were found to be very similar to the values calculated in the framework of the critical point symmetry X(5). In order to enable more stringent tests, including also absolute transition probabilities, two coincidence RDDS lifetime measurements were performed at the Laboratori Nazionali di Legnaro with the GASP spectrometer using the 152,154Sm(29Si,5n)176,178Os reactions. The deduced transition quadrupole moments in 178Os agree well with the X(5) predictions. For 176Os only preliminary results were obtained so far. These preliminary data support an X(5) like structure also in the case of 176Os. The experimental data of both nuclei are compared to calculations in the framework of the interacting boson model (IBM) and of the general collective model (GCM)

  7. Spectroscopy of the neutron-deficient isobars {sup 163}Re and {sup 163}W using tagging techniques

    SciTech Connect

    Joss, D. T.; Thomson, J.; Page, R. D.; Bianco, L.; Darby, I. G.; Grahn, T.; Pakarinen, J.; Paul, E. S.; Scholey, C.; Eeckhaudt, S.; Greenlees, P. T.; Jones, P. M.; Julin, R.; Juutinen, S.; Ketelhut, S.; Leino, M.; Leppaennen, A.-P.; Nyman, M.; Rahkila, P.; Sorri, J.

    2008-11-11

    Selective tagging techniques have been used to establish new band structures in the transitional isobars {sup 163}Re and {sup 163}W. These nuclei were produced in the {sup 106}Cd({sup 60}Ni, xp yn {gamma}) reaction at a bombarding energy of 270 MeV. Prompt {gamma} rays were detected at the target position using the JUROGAM spectrometer while recoiling ions were separated by the RITU separator and implanted into the GREAT spectrometer. At low spin, the yrast band of {sup 163}Re is shown to be a strongly coupled collective band based on a proton h{sub 11/2} configuration. In {sup 163}W, the decay path of the 13/2{sup +} isomeric state to the ground state has been identified and negative parity structures based on the ground state established.

  8. Study of neutron-deficient isotopes of Fl in the 239Pu, 240Pu + 48Ca reactions

    NASA Astrophysics Data System (ADS)

    Voinov, A. A.; Utyonkov, V. K.; Brewer, N. T.; Oganessian, Yu Ts; Rykaczewski, K. P.; Abdullin, F. Sh; Dmitriev, S. N.; Grzywacz, R. K.; Itkis, M. G.; Miernik, K.; Polyakov, A. N.; Roberto, J. B.; Sagaidak, R. N.; Shirokovsky, I. V.; Shumeiko, M. V.; Tsyganov, Yu S.; Subbotin, V. G.; Sukhov, A. M.; Sabelnikov, A. V.; Vostokin, G. K.; Hamilton, J. H.; Stoyer, M. A.; Strauss, S. Y.

    2016-07-01

    The results of the experiments aimed at the synthesis of Fl isotopes in the 239Pu + 48Ca and 240Pu + 48Ca reactions are presented. The experiment was performed using the Dubna gas-filled recoil separator at the U400 cyclotron. In the 239Pu+48Ca experiment one decay of spontaneously fissioning 284Fl was detected at 245-MeV beam energy. In the 240Pu+48Ca experiment three decay chains of 285Fl were detected at 245 MeV and four decays were assigned to 284Fl at the higher 48Ca beam energy of 250 MeV. The α-decay energy of 285Fl was measured for the first time and decay properties of its descendants 281Cn, 277Ds, 273Hs, 269Sg, and 265Rf were determined more precisely. The cross section of the 239Pu(48Ca,3n)284Fl reaction was observed to be about 20 times lower than those predicted by theoretical models and 50 times less than the value measured in the 244Pu+48Ca reaction. The cross sections of the 240Pu(48Ca,4-3n)284,285Fl at both 48Ca energies are similar and exceed that observed in the reaction with lighter isotope 239Pu by a factor of 10. The decay properties of the synthesized nuclei and their production cross sections indicate rapid decrease of stability of superheavy nuclei with departing from the neutron number N=184 predicted to be the next magic number.

  9. On the Relation between Stratospheric Chlorine/Bromine Loading and Short-Lived Tropospheric Source Gases. Appendix D

    NASA Technical Reports Server (NTRS)

    Ko, Malcolm K. W.; Sze, Nien-Dak; Scott, Courtney J.; Weisenstein, Debra K.

    1997-01-01

    Current methods for estimating the concentrations of inorganic chlorine/bromine species Cl(y)/Br(y) in the stratosphere due to decomposition of tropospheric source gases assume that the Cl(y)/Br(y) concentration in the stratosphere is determined mainly by the balance between production from in situ oxidation of the source gases in the stratosphere and removal by transport of Cl(y)/Br(y) out of the stratosphere. The rationale being that for source gases whose lifetimes are of the order of several months or longer the concentration of Cl(y)/Br(y) in the troposphere is small because they are produced at a relatively slow rate and also removed efficiently by washout processes. As a result of the small concentration, the rate at which Cl(y)/Br(y) is transported to the stratosphere is expected to be small compared to the in situ stratospheric production. Thus the transport of Cl(y)/Br(y) from the troposphere contributes little to the stratospheric concentration. In contrast, the origin of stratospheric Cl(y)/Br(y) from reactive source gases with tropospheric lifetimes comparable to the washout lifetime of Cl(y)/Br(y) (of the order of 10-30 days) in the troposphere is distinctly different. The in situ source in the stratosphere is expected to be significantly smaller because only a small portion of the source gas is expected to survive the troposphere to be transported into this region. At the same time these short-lived source gases produce appreciable amounts of Cl(y)/Br(y) in the troposphere such that transport to the stratosphere offers a larger source for stratospheric Cl(y)/Br(y) than in situ production. Thus, for reactive source species, simple methods of estimating the concentration of stratospheric Cl(y)/Br(y) that ignore the tropospheric contribution will seriously underestimate the loading. Therefore estimation of the stratospheric Cl(y)/Br(y) loading requires not only measurements of tropospheric source gases but also measurements of Cl(y)/Br(y) at the

  10. Application of mass spectrometric techniques for the trace analysis of short-lived iodine-containing volatiles emitted by seaweed.

    PubMed

    Kundel, Michael; Thorenz, Ute R; Petersen, Jan H; Huang, Ru-Jin; Bings, Nicolas H; Hoffmann, Thorsten

    2012-04-01

    Knowledge of the composition and emission rates of iodine-containing volatiles from major widespread seaweed species is important for modeling the impact of halogens on gas-phase atmospheric chemistry, new particle formation, and climate. In this work, we present the application of mass spectrometric techniques for the quantification of short-lived iodine-containing volatiles emitted by eight different seaweeds from the intertidal zone of Helgoland, Germany. A previously developed online time-of-flight aerosol mass spectrometric method was used to determine I(2) emission rates and investigate temporally resolved emission profiles. Simultaneously, iodocarbons were preconcentrated on solid adsorbent tubes and quantified offline using thermodesorption-gas chromatography-mass spectrometry. The total iodine content of the seaweeds was determined using microwave-assisted tetramethylammonium hydroxide extraction followed by inductively coupled-plasma mass spectrometry analysis. The highest total iodine content was found in the Laminariales, followed by the brown algae Ascophyllum nodosum, Fucus vesiculosus, Fucus serratus, and both red algae Chondrus crispus and Delesseria sanguinea. Laminariales were found to be the strongest I(2) emitters. Time series of the iodine release of Laminaria digitata and Laminaria hyperborea showed a strong initial I(2) emission when first exposed to air followed by an exponential decline of the release rate. For both species, I(2) emission bursts were observed. For Laminaria saccharina und F. serratus, a more continuous I(2) release profile was detected, however, F. serratus released much less I(2). A. nodosum and F. vesiculosus showed a completely different emission behavior. The I(2) emission rates of these species were slowly increasing with time during the first 1 to 2 h until a more or less stable I(2) emission rate was reached. The lowest I(2) emission rates were detected for the red algae C. crispus and D. sanguinea. Total iodocarbon

  11. Comment on 'Electron-induced bond breaking at low energies in HCOOH and glycine: The role of very short-lived {sigma}* anion states'

    SciTech Connect

    Rescigno, T. N.; Trevisan, C. S.; Orel, A. E.

    2009-10-15

    Recent model calculations by Gallup et al. [Phys. Rev. A79, 042710 (2009)] suggest that low-energy dissociative electron attachment to formic acid can be explained solely in terms of a very short-lived {sigma}* anion state and that no {sigma}*/{pi}* coupling is required. We argue that this interpretation of the experimental data, which is at odds with our earlier study, is flawed.

  12. Study of near-stability nuclei populated as fission fragments in heavy-ion fusion reactions

    SciTech Connect

    Fotiadis, Nikolaos; Nelson, Ronald O; Devlin, Matthew; Cizewski, Jolie A; Krucken, Reiner; Clark, R M; Fallon, Paul; Lee, I Yang; Macchiavelli, Agusto O; Becker, John A; Younes, Walid

    2010-01-01

    Examples are presented to illustrate the power of prompt {gamma}-ray spectroscopy of fission fragments from compound nuclei with A {approx} 200 formed in fusion-evaporation reactions in experiments using the Gammasphere Ge-detector array. Complementary methods, such as Coulomb excitation and deep-inelastic processes, are also discussed. In other cases (n, xn{gamma}) reactions on stable isotopes have been used to establish neutron excitation functions for {gamma}-rays using a pulsed 'white'-neutron source, coupled to a high-energy-resolution germanium-detector array. The excitation functions can unambiguously assign {gamma}-rays to a specific reaction product. Results from all these methods bridge the gaps in the systematics of high-spin states between the neutron-deficient and neutron-rich nuclei. Results near shell closures should motivate new shell model calculations.

  13. Drag on a Satellite Moving across a Spherical Galaxy: Tidal and Frictional Forces in Short-lived Encounters

    NASA Astrophysics Data System (ADS)

    Colpi, Monica; Pallavicini, Andrea

    1998-07-01

    The drag force on a satellite of mass M moving with speed V in the gravitational field of a spherically symmetric background of stars is computed. During the encounter, the stars are subject to a time-dependent force that alters their equilibrium. The resulting distortion in the stellar density field acts back to produce a force FΔ that decelerates the satellite. This force is computed using a perturbative technique known as linear response theory. In this paper, we extend the formalism of linear response to derive the correct expression for the back-reaction force FΔ that applies when the stellar system is described by an equilibrium one-particle distribution function. FΔ is expressed in terms of a suitable correlation function that couples the satellite dynamics to the unperturbed dynamics of the stars. At time t, the force depends upon the whole history of the composite system. In the formalism, we account for the shift of the stellar center of mass resulting from linear momentum conservation. The self-gravity of the response is neglected since it contributes to a higher order in the perturbation. Linear response theory applies also to the case of a satellite orbiting outside the spherical galaxy. The case of a satellite moving on a straight line, at high speed relative to the stellar dispersion velocity, is explored. We find that the satellite during its passage raises (1) global tides in the stellar distribution and (2) a wake, i.e., an overdense region behind its trail. If the satellite motion is external to the galaxy, it suffers a dissipative force that is not exclusively acting along V but acquires a component along R, the position vector relative to the center of the spherical galaxy. We derive the analytical expression of the force in the impulse approximation. In penetrating short-lived encounters, the satellite moves across the stellar distribution and the transient wake excited in the density field is responsible for most of the deceleration. We

  14. Cosmogenic nuclei

    NASA Technical Reports Server (NTRS)

    Raisbeck, G. M.

    1986-01-01

    Cosmogenic nuclei, nuclides formed by nuclear interactions of galactic and solar cosmic rays with extraterrestrial or terrestrial matter are discussed. Long lived radioactive cosmogenic isotopes are focused upon. Their uses in dating, as tracers of the interactions of cosmic rays with matter, and in obtaining information on the variation of primary cosmic ray flux in the past are discussed.

  15. Pushing the relative mass accuracy limit of ISOLTRAP on exotic nuclei below 10 ppb

    NASA Astrophysics Data System (ADS)

    Blaum, K.; Beck, D.; Bollen, G.; Herfurth, F.; Kellerbauer, A.; Kluge, H.-J.; Moore, R. B.; Sauvan, E.; Scheidenberger, C.; Schwarz, S.; Schweikhard, L.

    2003-05-01

    The Penning trap mass spectrometer ISOLTRAP plays a leading role in mass spectrometry of short-lived nuclides. The recent installation of a radio-frequency quadrupole trap and a carbon cluster ion source allowed for the first time mass measurements on exotic nuclei with a relative uncertainty of δ m/ m≈1×10 -8. The status of ISOLTRAP mass spectrometry and recent highlights are presented.

  16. Novel internal target for electron scattering off unstable nuclei.

    PubMed

    Wakasugi, M; Emoto, T; Furukawa, Y; Ishii, K; Ito, S; Koseki, T; Kurita, K; Kuwajima, A; Masuda, T; Morikawa, A; Nakamura, M; Noda, A; Ohnishi, T; Shirai, T; Suda, T; Takeda, H; Tamae, T; Tongu, H; Wang, S; Yano, Y

    2008-04-25

    A novel internal target has been developed, which will make electron scattering off short-lived radioactive nuclei possible in an electron storage ring. An "ion trapping" phenomenon in the electron storage ring was successfully utilized for the first time to form the target for electron scattering. Approximately 7 x 10(6) stable 133Cs ions were trapped along the electron beam axis for 85 ms at an electron beam current of 80 mA. The collision luminosity between the stored electrons and trapped Cs ions was determined to be 2.4(8) x 10(25) cm(-2) s(-1) by measuring elastically scattered electrons. PMID:18518208

  17. Species Selection Favors Dispersive Life Histories in Sea Slugs, but Higher Per-Offspring Investment Drives Shifts to Short-Lived Larvae.

    PubMed

    Krug, Patrick J; Vendetti, Jann E; Ellingson, Ryan A; Trowbridge, Cynthia D; Hirano, Yayoi M; Trathen, Danielle Y; Rodriguez, Albert K; Swennen, Cornelis; Wilson, Nerida G; Valdés, Ángel A

    2015-11-01

    For 40 years, paleontological studies of marine gastropods have suggested that species selection favors lineages with short-lived (lecithotrophic) larvae, which are less dispersive than long-lived (planktotrophic) larvae. Although lecithotrophs appeared to speciate more often and accumulate over time in some groups, lecithotrophy also increased extinction rates, and tests for state-dependent diversification were never performed. Molecular phylogenies of diverse groups instead suggested lecithotrophs accumulate without diversifying due to frequent, unidirectional character change. Although lecithotrophy has repeatedly originated in most phyla, no adult trait has been correlated with shifts in larval type. Thus, both the evolutionary origins of lecithotrophy and its consequences for patterns of species richness remain poorly understood. Here, we test hypothesized links between development mode and evolutionary rates using likelihood-based methods and a phylogeny of 202 species of gastropod molluscs in Sacoglossa, a clade of herbivorous sea slugs. Evolutionary quantitative genetics modeling and stochastic character mapping supported 27 origins of lecithotrophy. Tests for correlated evolution revealed lecithotrophy evolved more often in lineages investing in extra-embryonic yolk, the first adult trait associated with shifts in development mode across a group. However, contrary to predictions from paleontological studies, species selection actually favored planktotrophy; most extant lecithotrophs originated through recent character change, and did not subsequently diversify. Increased offspring provisioning in planktotrophs thus favored shifts to short-lived larvae, which led to short-lived lineages over macroevolutionary time scales. These findings challenge long-standing assumptions about the effects of alternative life histories in the sea. Species selection can explain the long-term persistence of planktotrophy, the ancestral state in most clades, despite frequent

  18. Climate response to projected changes in short-lived species under an A1B scenario from 2000-2050 in the GISS climate model

    SciTech Connect

    Menon, Surabi; Shindell, Drew T.; Faluvegi, Greg; Bauer, Susanne E.; Koch, Dorothy M.; Unger, Nadine; Menon, Surabi; Miller, Ron L.; Schmidt, Gavin A.; Streets, David G.

    2007-03-26

    We investigate the climate forcing from and response to projected changes in short-lived species and methane under the A1B scenario from 2000-2050 in the GISS climate model. We present a meta-analysis of new simulations of the full evolution of gas and aerosol species and other existing experiments with variations of the same model. The comparison highlights the importance of several physical processes in determining radiative forcing, especially the effect of climate change on stratosphere-troposphere exchange, heterogeneous sulfate-nitrate-dust chemistry, and changes in methane oxidation and natural emissions. However, the impact of these fairly uncertain physical effects is substantially less than the difference between alternative emission scenarios for all short-lived species. The net global mean annual average direct radiative forcing from the short-lived species is .02 W/m{sup 2} or less in our projections, as substantial positive ozone forcing is largely offset by negative aerosol direct forcing. Since aerosol reductions also lead to a reduced indirect effect, the global mean surface temperature warms by {approx}0.07 C by 2030 and {approx}0.13 C by 2050, adding 19% and 17%, respectively, to the warming induced by long-lived greenhouse gases. Regional direct forcings are large, up to 3.8 W/m{sup 2}. The ensemble-mean climate response shows little regional correlation with the spatial pattern of the forcing, however, suggesting that oceanic and atmospheric mixing generally overwhelms the effect of even large localized forcings. Exceptions are the polar regions, where ozone and aerosols may induce substantial seasonal climate changes.

  19. Daily variation of radon gas and its short-lived progeny concentration near ground level and estimation of aerosol residence time

    NASA Astrophysics Data System (ADS)

    M, Mohery; A, M. Abdallah; A, Ali; S, S. Baz

    2016-05-01

    Atmospheric concentrations of radon (222Rn) gas and its short-lived progenies 218Po, 214Pb, and 214Po were continuously monitored every four hours at the ground level in Jeddah city, Kingdom of Saudi Arabia. The measurements were performed three times every week, starting from November 2014 to October 2015. A method of electrostatic precipitation of positively charged 218Po and 214Po by a positive voltage was applied for determining 222Rn gas concentration. The short-lived 222Rn progeny concentration was determined by using a filter holder connected with the alpha-spectrometric technique. The meteorological parameters (relative air humidity, air temperature, and wind speed) were determined during the measurements of 222Rn and its progeny concentrations. 222Rn gas as well as its short-lived progeny concentration display a daily and seasonal variation with high values in the night and early morning hours as compared to low values at noon and in the afternoon. The observed monthly atmospheric concentrations showed a seasonal trend with the highest values in the autumn/winter season and the lowest values in the spring/summer season. Moreover, and in parallel with alpha-spectrometric measurements, a single filter-holder was used to collect air samples. The deposited activities of 214Pb and the long-lived 222Rn daughter 210Pb on the filter were measured with the gamma spectrometric technique. The measured activity concentrations of 214Pb by both techniques were found to be relatively equal largely. The highest mean seasonally activity concentrations of 210Pb were observed in the autumn/winter season while the lowest mean were observed in the spring/summer season. The mean residence time (MRT) of aerosol particles in the atmospheric air could be estimated from the activity ratios of 210Pb/214Pb. Project supported by the Deanship of Scientific Research (DSR), King Abdulaziz University, Jeddah (Grant No. 291/965/1434).

  20. Freshly induced short-lived gamma-ray activity as a measure of fission rates in lightly re-irradiated spent fuel

    NASA Astrophysics Data System (ADS)

    Kröhnert, H.; Perret, G.; Murphy, M. F.; Chawla, R.

    2010-12-01

    A new measurement technique has been developed to determine fission rates in burnt fuel, following re-irradiation in a zero-power research reactor. The development has been made in the frame of the LIFE@PROTEUS program at the Paul Scherrer Institute, which aims at characterizing the interfaces between fresh and highly burnt fuel assemblies in modern LWRs. To discriminate against the high intrinsic gamma-ray activity of the burnt fuel, the proposed measurement technique uses high-energy gamma-rays, above 2000 keV, emitted by short-lived fission products freshly produced in the fuel. To demonstrate the feasibility of this technique, a fresh UO 2 sample and a 36 GWd/t burnt UO 2 sample were irradiated in the PROTEUS reactor and their gamma-ray activities were recorded directly after irradiation. For both fresh and the burnt fuel samples, relative fission rates were derived for different core positions, based on the short-lived 142La (2542 keV), 89Rb (2570 keV), 138Cs (2640 keV) and 95Y (3576 keV) gamma-ray lines. Uncertainties on the inter-position fission rate ratios were mainly due to the uncertainties on the net-area of the gamma-ray peaks and were about 1-3% for the fresh sample, and 3-6% for the burnt one. Thus, for the first time, it has been shown that the short-lived gamma-ray activity, induced in burnt fuel by irradiation in a zero-power reactor, can be used as a quantitative measure of the fission rate. For both fresh and burnt fuel, the measured results agreed, within the uncertainties, with Monte Carlo (MCNPX) predictions.

  1. 182Hf–182W age dating of a 26Al-poor inclusion and implications for the origin of short-lived radioisotopes in the early Solar System

    PubMed Central

    Holst, Jesper C.; Olsen, Mia B.; Paton, Chad; Nagashima, Kazuhide; Schiller, Martin; Wielandt, Daniel; Larsen, Kirsten K.; Connelly, James N.; Jørgensen, Jes K.; Krot, Alexander N.; Nordlund, Åke; Bizzarro, Martin

    2013-01-01

    Refractory inclusions [calcium–aluminum-rich inclusions, (CAIs)] represent the oldest Solar System solids and provide information regarding the formation of the Sun and its protoplanetary disk. CAIs contain evidence of now extinct short-lived radioisotopes (e.g., 26Al, 41Ca, and 182Hf) synthesized in one or multiple stars and added to the protosolar molecular cloud before or during its collapse. Understanding how and when short-lived radioisotopes were added to the Solar System is necessary to assess their validity as chronometers and constrain the birthplace of the Sun. Whereas most CAIs formed with the canonical abundance of 26Al corresponding to 26Al/27Al of ∼5 × 10−5, rare CAIs with fractionation and unidentified nuclear isotope effects (FUN CAIs) record nucleosynthetic isotopic heterogeneity and 26Al/27Al of <5 × 10−6, possibly reflecting their formation before canonical CAIs. Thus, FUN CAIs may provide a unique window into the earliest Solar System, including the origin of short-lived radioisotopes. However, their chronology is unknown. Using the 182Hf–182W chronometer, we show that a FUN CAI recording a condensation origin from a solar gas formed coevally with canonical CAIs, but with 26Al/27Al of ∼3 × 10−6. The decoupling between 182Hf and 26Al requires distinct stellar origins: steady-state galactic stellar nucleosynthesis for 182Hf and late-stage contamination of the protosolar molecular cloud by a massive star(s) for 26Al. Admixing of stellar-derived 26Al to the protoplanetary disk occurred during the epoch of CAI formation and, therefore, the 26Al–26Mg systematics of CAIs cannot be used to define their formation interval. In contrast, our results support 182Hf homogeneity and chronological significance of the 182Hf–182W clock. PMID:23671077

  2. 182Hf-182W age dating of a 26Al-poor inclusion and implications for the origin of short-lived radioisotopes in the early Solar System.

    PubMed

    Holst, Jesper C; Olsen, Mia B; Paton, Chad; Nagashima, Kazuhide; Schiller, Martin; Wielandt, Daniel; Larsen, Kirsten K; Connelly, James N; Jørgensen, Jes K; Krot, Alexander N; Nordlund, Ake; Bizzarro, Martin

    2013-05-28

    Refractory inclusions [calcium-aluminum-rich inclusions, (CAIs)] represent the oldest Solar System solids and provide information regarding the formation of the Sun and its protoplanetary disk. CAIs contain evidence of now extinct short-lived radioisotopes (e.g., (26)Al, (41)Ca, and (182)Hf) synthesized in one or multiple stars and added to the protosolar molecular cloud before or during its collapse. Understanding how and when short-lived radioisotopes were added to the Solar System is necessary to assess their validity as chronometers and constrain the birthplace of the Sun. Whereas most CAIs formed with the canonical abundance of (26)Al corresponding to (26)Al/(27)Al of ∼5 × 10(-5), rare CAIs with fractionation and unidentified nuclear isotope effects (FUN CAIs) record nucleosynthetic isotopic heterogeneity and (26)Al/(27)Al of <5 × 10(-6), possibly reflecting their formation before canonical CAIs. Thus, FUN CAIs may provide a unique window into the earliest Solar System, including the origin of short-lived radioisotopes. However, their chronology is unknown. Using the (182)Hf-(182)W chronometer, we show that a FUN CAI recording a condensation origin from a solar gas formed coevally with canonical CAIs, but with (26)Al/(27)Al of ∼3 × 10(-6). The decoupling between (182)Hf and (26)Al requires distinct stellar origins: steady-state galactic stellar nucleosynthesis for (182)Hf and late-stage contamination of the protosolar molecular cloud by a massive star(s) for (26)Al. Admixing of stellar-derived (26)Al to the protoplanetary disk occurred during the epoch of CAI formation and, therefore, the (26)Al-(26)Mg systematics of CAIs cannot be used to define their formation interval. In contrast, our results support (182)Hf homogeneity and chronological significance of the (182)Hf-(182)W clock. PMID:23671077

  3. Short-lived 244Pu points to compact binary mergers as sites for heavy r-process nucleosynthesis

    NASA Astrophysics Data System (ADS)

    Hotokezaka, Kenta; Piran, Tsvi; Paul, Michael

    2015-12-01

    The origin of heavy elements produced through rapid neutron capture (`r-process’) by seed nuclei is one of the current nucleosynthesis mysteries. Core collapse supernovae (cc-SNe; ref. ) and compact binary mergers are considered as possible sites. The first produces small amounts of material at a high event rate whereas the latter produces large amounts in rare events. Radioactive elements with the right lifetime can break the degeneracy between high-rate/low-yield and low-rate/high-yield scenarios. Among radioactive elements, most interesting is 244Pu (half-life of 81 million years), for which both the current accumulation of live 244Pu particles accreted via interstellar particles in the Earth’s deep-sea floor and the Early Solar System (ESS) abundances have been measured. Interestingly, the estimated 244Pu abundance in the current interstellar medium inferred from deep-sea measurements is significantly lower than that corresponding to the ESS measurements. Here we show that both the current and ESS abundances of 244Pu are naturally explained within the low-rate/high-yield scenario. The inferred event rate remarkably agrees with compact binary merger rates estimated from Galactic neutron star binaries and from short gamma-ray bursts. Furthermore, the ejected mass of r-process elements per event agrees with both theoretical and observational macronova/kilonova estimates.

  4. First results using a new technology for measuring masses of very short-lived nuclides with very high accuracy: The MISTRAL program at ISOLDE

    SciTech Connect

    Monsanglant, C.; Audi, G.; Conreur, G.; Cousin, R.; Doubre, H.; Jacotin, M.; Henry, S.; Kepinski, J.-F.; Lunney, D.; Saint Simon, M. de; Thibault, C.; Toader, C.; Bollen, G.; Lebee, G.; Scheidenberger, C.; Borcea, C.; Duma, M.; Kluge, H.-J.; Le Scornet, G.

    1999-11-16

    MISTRAL is an experimental program to measure masses of very short-lived nuclides (T{sub 1/2} down to a few ms), with a very high accuracy (a few 10{sup -7}). There were three data taking periods with radioactive beams and 22 masses of isotopes of Ne, Na, Mg, Al, K, Ca, and Ti were measured. The systematic errors are now under control at the level of 8x10{sup -7}, allowing to come close to the expected accuracy. Even for the very weakly produced {sup 30}Na (1 ion at the detector per proton burst), the final accuracy is 7x10{sup -7}.

  5. Towards a novel laser-driven method of exotic nuclei extraction-acceleration for fundamental physics and technology

    NASA Astrophysics Data System (ADS)

    Nishiuchi, M.; Sakaki, H.; Esirkepov, T. Zh.; Nishio, K.; Pikuz, T. A.; Faenov, A. Ya.; Skobelev, I. Yu.; Orlandi, R.; Pirozhkov, A. S.; Sagisaka, A.; Ogura, K.; Kanasaki, M.; Kiriyama, H.; Fukuda, Y.; Koura, H.; Kando, M.; Yamauchi, T.; Watanabe, Y.; Bulanov, S. V.; Kondo, K.; Imai, K.; Nagamiya, S.

    2016-04-01

    A combination of a petawatt laser and nuclear physics techniques can crucially facilitate the measurement of exotic nuclei properties. With numerical simulations and laser-driven experiments we show prospects for the Laser-driven Exotic Nuclei extraction-acceleration method proposed in [M. Nishiuchi et al., Phys, Plasmas 22, 033107 (2015)]: a femtosecond petawatt laser, irradiating a target bombarded by an external ion beam, extracts from the target and accelerates to few GeV highly charged short-lived heavy exotic nuclei created in the target via nuclear reactions.

  6. Short-lived species detection of nitrous acid by external-cavity quantum cascade laser based quartz-enhanced photoacoustic absorption spectroscopy

    NASA Astrophysics Data System (ADS)

    Yi, Hongming; Maamary, Rabih; Gao, Xiaoming; Sigrist, Markus W.; Fertein, Eric; Chen, Weidong

    2015-03-01

    Spectroscopic detection of short-lived gaseous nitrous acid (HONO) at 1254.85 cm-1 was realized by off-beam coupled quartz-enhanced photoacoustic spectroscopy (QEPAS) in conjunction with an external cavity quantum cascade lasers (EC-QCL). High sensitivity monitoring of HONO was performed within a very small gas-sample volume (of ˜40 mm3) allowing a significant reduction (of about 4 orders of magnitude) of air sampling residence time which is highly desired for accurate quantification of chemically reactive short-lived species. Calibration of the developed QEPAS-based HONO sensor was carried out by means of lab-generated HONO samples whose concentrations were determined by direct absorption spectroscopy involving a ˜109.5 m multipass cell and a distributed feedback QCL. A minimum detection limit (MDL) of 66 ppbv (1 σ) HONO was achieved at 70 mbar using a laser output power of 50 mW and 1 s integration time, which corresponded to a normalized noise equivalent absorption coefficient of 3.6 × 10-8 cm-1 W/Hz1/2. This MDL was down to 7 ppbv at the optimal integration time of 150 s. The corresponding 1σ minimum detected absorption coefficient is ˜1.1 × 10-7 cm-1 (MDL ˜ 3 ppbv) in 1 s and ˜1.1 × 10-8 cm-1 (MDL ˜ 330 pptv) in 150 s, respectively, with 1 W laser power.

  7. Exotic Nuclei

    SciTech Connect

    Galindo-Uribarri, Alfredo {nmn}

    2010-01-01

    Current experimental developments on the study of exotic nuclei far from the valley of stability are discussed. I start with general aspects related to the production of radioactive beams followed by the description of some of the experimental tools and specialized techniques for studies in reaction spectroscopy, nuclear structure research and nuclear applications with examples from selected topical areas with which I have been involved. I discuss some of the common challenges faced in Accelerator Mass Spectrometry (AMS) and Radioactive Ion Beam (RIB) science.

  8. Studies of neutron-rich nuclei far from stability at TRISTAN

    SciTech Connect

    Gill, R.L.

    1984-01-01

    The ISOL facility, TRISTAN, is a user facility located at Brookhaven National Laboratory's High Flux Beam Reactor. Short-lived, neutron-rich nuclei, far from stability, are produced by thermal neutron fission of /sup 235/U. An extensive array of experimental end stations are available for nuclear structure studies. These studies are augmented by a variety of long-lived ion sources suitable for use at a reactor facility. Some recent results at TRISTAN are presented as examples of using an ISOL facility to study series of nuclei, whereby an effective means of conducting nuclear structure investigations is available.

  9. Development of a system for real-time measurements of metabolite transport in plants using short-lived positron-emitting radiotracers

    NASA Astrophysics Data System (ADS)

    Kiser, Matthew R.

    Over the past 200 years, the Earth's atmospheric carbon dioxide (CO 2) concentration has increased by more than 35%, and climate experts predict that CO2 levels may double by the end of this century. Understanding the mechanisms of resource management in plants is fundamental for predicting how plants will respond to the increase in atmospheric CO 2. Plant productivity sustains life on Earth and is a principal component of the planet's system that regulates atmospheric CO2 concentration. As such, one of the central goals of plant science is to understand the regulatory mechanisms of plant growth in a changing environment. Short-lived positron-emitting radiotracer techniques provide time-dependent data that are critical for developing models of metabolite transport and resource distribution in plants and their microenvironments. To better understand the effects of environmental changes on resource transport and allocation in plants, we have developed a system for real-time measurements of rnetabolite transport in plants using short-lived positron-emitting radio-tracers. This thesis project includes the design, construction, and demonstration of the capabilities of this system for performing real-time measurements of metabolite transport in plants. The short-lived radiotracer system described in this dissertation takes advantage of the combined capabilities and close proximity of two research facilities at. Duke University: the Triangle Universities Nuclear Laboratory (TUNL) and the Duke University Phytotron, which are separated by approximately 100 meters. The short-lived positron-emitting radioisotopes are generated using the 10-MV tandem Van de Graaff accelerator located in the main TUNL building, which provides the capability of producing short-lived positron-emitting isotopes such as carbon-11 (11C: 20 minute half-life), nitrogen-13 (13N; 10 minute half-life), fluorine-18 (18F; 110 minute half-life), and oxygen-15 (15O; 2 minute half-life). The radioisotopes may

  10. Development of a system for real-time measurements of metabolite transport in plants using short-lived positron-emitting radiotracers

    NASA Astrophysics Data System (ADS)

    Kiser, Matthew R.

    Over the past 200 years, the Earth's atmospheric carbon dioxide (CO 2) concentration has increased by more than 35%, and climate experts predict that CO2 levels may double by the end of this century. Understanding the mechanisms of resource management in plants is fundamental for predicting how plants will respond to the increase in atmospheric CO 2. Plant productivity sustains life on Earth and is a principal component of the planet's system that regulates atmospheric CO2 concentration. As such, one of the central goals of plant science is to understand the regulatory mechanisms of plant growth in a changing environment. Short-lived positron-emitting radiotracer techniques provide time-dependent data that are critical for developing models of metabolite transport and resource distribution in plants and their microenvironments. To better understand the effects of environmental changes on resource transport and allocation in plants, we have developed a system for real-time measurements of rnetabolite transport in plants using short-lived positron-emitting radio-tracers. This thesis project includes the design, construction, and demonstration of the capabilities of this system for performing real-time measurements of metabolite transport in plants. The short-lived radiotracer system described in this dissertation takes advantage of the combined capabilities and close proximity of two research facilities at. Duke University: the Triangle Universities Nuclear Laboratory (TUNL) and the Duke University Phytotron, which are separated by approximately 100 meters. The short-lived positron-emitting radioisotopes are generated using the 10-MV tandem Van de Graaff accelerator located in the main TUNL building, which provides the capability of producing short-lived positron-emitting isotopes such as carbon-11 (11C: 20 minute half-life), nitrogen-13 (13N; 10 minute half-life), fluorine-18 (18F; 110 minute half-life), and oxygen-15 (15O; 2 minute half-life). The radioisotopes may

  11. Octupole shaps in nuclei, and some rotational consequences thereof

    SciTech Connect

    Nazarewicz, W.; Olanders, P.; Ragnarsson, I.; Dudek, J.; Leander, G.A.

    1984-01-01

    During the last years a large number of experimental papers presenting spectroscopic evidence for collective dipole and octupole deformations have appeared. Many theoretical attempts have been made to explain the observed spectroscopic properties in terms of stable octupole deformations. The coupling by the octupole potential, being proportional to Y/sub 30/, is strongest for those subshells for which ..delta..1 = 3. Therefore the tendency towards octupole deformation occurs just beyond closed shells where the high-j intruder subshells (N,1,j) lie very close to the normal parity subshells (N-1,1-3,j-3), i.e. for the particle numbers 34 (g/sub 9/2/-p/sub 3/2/), 56 (h/sub 11/2/-d/sub 5/2/). 9C (i/sub 13/2/-f/sub 7/2/) and 134 (j/sub 15/2/-g/sub 9/2/). Empirically, it is specifically for the particle numbers listed above that negative parity states are observed at relatively low energies in doubly even nuclei. From the different combinations of octupole-driving particle numbers four regions of likely candidates for octupole deformed equilibrium shapes emerge, namely the neutron-deficient nuclei with Z approx. = 90, N approx. = 134 (light actinides) and Z approx. = 34, N approx. = 34 (A approx. = 70) and the neutron-rich nuclei with Z approx. = 56, N approx. = 90 (heavy Ba) and Z approx. = 34, N/sup 56/ (A approx. = 90). In our calculations we searched for octupole unstable nuclei in these four mass regions. The Strutinsky method with the deformed Woods-Saxon potential was employed. The macroscopic part consists of a finite-range liquid drop energy, where both the surface and Coulomb terms contain a diffuseness correction.

  12. Detection of 210Po on filter papers 16 years after use for the collection of short-lived radon progeny in a room.

    PubMed

    Abu-Jarad, F; Fazal-ur-Rehman

    2003-01-01

    Radon gas was allowed to accumulate in its radium source and then injected into a 36 m(3) test room, resulting in an initial radon concentration of 15 kBq m(-3). Filter papers were used to collect the short-lived radon progeny and thus to measure the Potential Alpha Energy Concentration (PAEC) in-situ in the year 1984 at different times and conditions according to the experimental design. The radon progeny collected on the filter papers were studied as a function of aerosol particle concentration ranging from 10(2)-10(5) particles cm(-3) in three different experiments. The highest aerosol particle concentration was generated by indoor cigarette smoking. Those filters were stored after the experiment, and were used after 16 years to study the activity of the radon long-lived alpha emitter progeny, (210)Po (T(1/2)=138 days). This isotope is separated from the short-lived progeny by (210)Pb beta emitter with 22.3 years half-life. After 16 years' storage of these filters, each filter paper was sandwiched and wrapped between two CR-39 nuclear track detectors, to put the detectors in contact with the surfaces of different filters, for 337 days. Correlation between the PAEC measured using filter papers in the year 1984 and the activity of long-lived alpha emitter (210)Po on the same filter papers measured in the year 2000 were studied. The results of the (210)Po activity showed a very good correlation of 0.92 with the PAEC 16 years ago. The results also depict that the PAEC and (210)Po activity in indoor air increased with the increase of aerosol particle concentration, which shows the attachment of short-lived radon progeny with the aerosol particles. The experiment proves that indoor cigarette smoking is a major source of aerosol particles carrying radon progeny and, thus, indoor cigarette smoking is an additional source of internal radiation hazard to the occupants whether smoker or non-smoker. PMID:12633999

  13. First Results Using a New Technology for Measuring Masses of Very Short-Lived Nuclides with Very High Accuracy: the MISTRAL Program at ISOLDE

    SciTech Connect

    C. Monsanglant; C. Toader; G. Audi; G. Bollen; C. Borcea; G. Conreur; R. Cousin; H. Doubre; M. Duma; M. Jacotin; S. Henry; J.-F. Kepinski; H.-J. Kluge; G. Lebee; G. Le Scornet; D. Lunney; M. de Saint Simon; C. Scheidenberger; C. Thibault

    1999-12-31

    MISTRAL is an experimental program to measure masses of very short-lived nuclides (T{sub 1/2} down to a few ms), with a very high accuracy (a few 10{sup -7}). There were three data taking periods with radioactive beams and 22 masses of isotopes of Ne, Na{clubsuit}, Mg, Al{clubsuit}, K, Ca, and Ti were measured. The systematic errors are now under control at the level of 8x10{sup -7}, allowing to come close to the expected accuracy. Even for the very weakly produced {sup 30}Na (1 ion at the detector per proton burst), the final accuracy is 7x10{sup -7}.

  14. Neutron activation analysis for Dy, Hf, Rb, Sc and Se in some Ghanaian cereals and vegetables using short-lived nuclides and Compton suppression spectrometry.

    PubMed

    Nyarko, B J B; Akaho, E H K; Fletcher, J J; Chatt, A

    2008-08-01

    A pseudo-cyclic instrumental neutron activation analysis (PCINAA) method has been developed to determine selected elements in various types of cereal and vegetable from Ghana using relatively short-lived nuclides (t1/2<80 s) and the Compton suppression counting. The samples were irradiated for 10 s at the Dalhousie University SLOWPOKE-2 research reactor facility (DUSR) and allowed to decay for 20 s, and counted for 40 s. The process is repeated every 50 s for 4 cycles to quantify Dy, Hf, Rb, Sc and Se through 165mDy, 179Hf, 86mRb, 46mSc, and 77mSe. The detection limits were generally of the order of 1.0 ng g(-1) except for Rb which is about 1 microg g(-1). Both precision and accuracy of the method were found to be good. PMID:18424050

  15. Design a 10 kJ IS Mather Type Plasma Focus for Solid Target Activation to Produce Short-Lived Radioisotopes 12C(d,n)13N

    NASA Astrophysics Data System (ADS)

    Sadat Kiai, S. M.; Adlparvar, S.; Sheibani, S.; Elahi, M.; Safarien, A.; Farhangi, S.; Zirak, A. R.; Alhooie, S.; Mortazavi, B. N.; Khalaj, M. M.; Khanchi, A. R.; Dabirzadeh, A. A.; Kashani, A.; Zahedi, F.

    2010-10-01

    A 10 kJ (15 kV, 88 μF) IS (Iranian Sun) Mather type plasma focus device has been studied to determine the activity of a compound exogenous carbon solid target through 12C(d,n)13N nuclear reaction. The produced 13N is a short-lived radioisotope with a half-life of 9.97 min and threshold energy of 0.28 MeV. The results indicate that energetic deuterons impinging on the solid target can produce yield of = 6.7 × 10-5 with an activity of A = 6.8 × 104 Bq for one plasma focus shut and A ν = 4 × 105 Bq for 6 shut per mint when the projectile maximum deuterons energy is E max = 3 MeV.

  16. Osteosarcoma risk after simultaneous incorporation of the long-lived radionuclide sup 227 Ac and the short-lived radionuclide sup 227 Th

    SciTech Connect

    Mueller, W.A.M.; Murray, A.B.; Linzner, U.; Luz, A. )

    1990-01-01

    The effect of injection of 1.85 kBq/kg of the long-lived radionuclide {sup 227}Ac on the induction of osteosarcomas in female NMRI mice by different dose levels (18.5, 74, and 185 kBq/kg) of the short-lived radionuclide {sup 227}Th was investigated. The highest absolute osteosarcoma incidence was observed with the highest doses of {sup 227}Th. Addition of {sup 227}Ac resulted in an additional osteosarcoma incidence only at the lowest dose of {sup 227}Th and did not affect the osteosarcoma incidence resulting from higher doses of {sup 227}Th. The longest times to tumor appearance were observed with {sup 227}Ac alone. The latent period in two different age groups (4 weeks and 10-12 weeks) appeared to be similar following injection with combined doses of {sup 227}Th and {sup 227}Ac but different after injection of each radionuclide alone.

  17. The Effect of Observers’ Mood on the Local Processing of Emotional Faces: Evidence from Short-Lived and Prolonged Mood States

    PubMed Central

    Mokhtari, Setareh; Buttle, Heather

    2015-01-01

    We examined the effect of induced mood, varying in valence and longevity, on local processing of emotional faces. It was found that negative facial expression conveyed by the global level of the face interferes with efficient processing of the local features. The results also showed that the duration of involvement with a mood influenced the local processing. We observed that attending to the local level of faces is not different in short-lived happy and sad mood states. However, as the mood state is experienced for a longer period, local processing was impaired in happy mood compared to sad mood. Taken together, we concluded that both facial expressions and affective states influence processing of the local parts of faces. Moreover, we suggest that mediating factors like the duration of involvement with the mood play a role in the interrelation between mood, attention, and perception. PMID:25883696

  18. Triggering collapse of the presolar dense cloud core and injecting short-lived radioisotopes with a shock wave. III. Rotating three-dimensional cloud cores

    SciTech Connect

    Boss, Alan P.; Keiser, Sandra A.

    2014-06-10

    A key test of the supernova triggering and injection hypothesis for the origin of the solar system's short-lived radioisotopes is to reproduce the inferred initial abundances of these isotopes. We present here the most detailed models to date of the shock wave triggering and injection process, where shock waves with varied properties strike fully three-dimensional, rotating, dense cloud cores. The models are calculated with the FLASH adaptive mesh hydrodynamics code. Three different outcomes can result: triggered collapse leading to fragmentation into a multiple protostar system; triggered collapse leading to a single protostar embedded in a protostellar disk; or failure to undergo dynamic collapse. Shock wave material is injected into the collapsing clouds through Rayleigh-Taylor fingers, resulting in initially inhomogeneous distributions in the protostars and protostellar disks. Cloud rotation about an axis aligned with the shock propagation direction does not increase the injection efficiency appreciably, as the shock parameters were chosen to be optimal for injection even in the absence of rotation. For a shock wave from a core-collapse supernova, the dilution factors for supernova material are in the range of ∼10{sup –4} to ∼3 × 10{sup –4}, in agreement with recent laboratory estimates of the required amount of dilution for {sup 60}Fe and {sup 26}Al. We conclude that a type II supernova remains as a promising candidate for synthesizing the solar system's short-lived radioisotopes shortly before their injection into the presolar cloud core by the supernova's remnant shock wave.

  19. Short-lived species detection of nitrous acid by external-cavity quantum cascade laser based quartz-enhanced photoacoustic absorption spectroscopy

    SciTech Connect

    Yi, Hongming; Maamary, Rabih; Fertein, Eric; Chen, Weidong; Gao, Xiaoming; Sigrist, Markus W.

    2015-03-09

    Spectroscopic detection of short-lived gaseous nitrous acid (HONO) at 1254.85 cm{sup −1} was realized by off-beam coupled quartz-enhanced photoacoustic spectroscopy (QEPAS) in conjunction with an external cavity quantum cascade lasers (EC-QCL). High sensitivity monitoring of HONO was performed within a very small gas-sample volume (of ∼40 mm{sup 3}) allowing a significant reduction (of about 4 orders of magnitude) of air sampling residence time which is highly desired for accurate quantification of chemically reactive short-lived species. Calibration of the developed QEPAS-based HONO sensor was carried out by means of lab-generated HONO samples whose concentrations were determined by direct absorption spectroscopy involving a ∼109.5 m multipass cell and a distributed feedback QCL. A minimum detection limit (MDL) of 66 ppbv (1 σ) HONO was achieved at 70 mbar using a laser output power of 50 mW and 1 s integration time, which corresponded to a normalized noise equivalent absorption coefficient of 3.6 × 10{sup −8 }cm{sup −1} W/Hz{sup 1/2}. This MDL was down to 7 ppbv at the optimal integration time of 150 s. The corresponding 1σ minimum detected absorption coefficient is ∼1.1 × 10{sup −7 }cm{sup −1} (MDL ∼ 3 ppbv) in 1 s and ∼1.1 × 10{sup −8 }cm{sup −1} (MDL ∼ 330 pptv) in 150 s, respectively, with 1 W laser power.

  20. Super-heavy nuclei with Z = 118 and their mass and charge spectrum of fission fragments

    NASA Astrophysics Data System (ADS)

    Maslyuk, V. T.; Smolyanyuk, A. V.

    2015-12-01

    The first results of the calculation of the mass and charge yields of fission fragments for over 60 isotopes which have Z = 118 are presented. The results were obtained from the condition of thermodynamic ordering of the ensemble of fission fragments. The role of neutrons shells with N = 82 or N = 126 and protons shells with Z = 50 in the realization of symmetric (or one-humped) and asymmetric (2- or 3-humped) shapes of the fission-fragment yields with the transition from neutron-proficient to neutron-deficient isotopes was investigated. The data of fragments yields had been analyzed under the conditions of a “cold” and “hot” fission. The calculations show the possibility to identify super-heavy nuclei with Z ≥ 118 produced synthetically by heavy-ion reaction on their mass/charge spectrum division.

  1. New Neutron Rich Nuclei Near {sup 208}Pb

    SciTech Connect

    Aeystoe, J.; Andreyev, A.; Evensen, A.-H.; Hoff, P.; Huhta, M.; Huyse, M.; ISOLDE Collaboration; Jokinen, A.; Karny, M.; Kugler, E.; Kurpeta, J.; Lettry, J.; Nieminen, A.; Plochocki, A.; Ramdhane, M.; Ravn, H.; Rykaczewski, K.; Szerypo, J.; VanDuppen, P.; Walter, G.; Woehr, A.

    1998-11-13

    The level properties near the stable doubly-magic nuclei formed the experimental grounds for the theoretical description of nuclear structure. However with a departure from the beta-stability line, the classical well-established shell structure might be modified. In particular, it may even vanish for extremely exotic neutron-rich nuclei near the neutron-drip line. Presently, it is impossible to verify such predictions by a direct experimental studies of these exotic objects. However, one may try to observe and understand the evolution of the nuclear structure while departing in the experiment as far as possible from the stable nuclei. An extension of experimental nuclear structure studies towards the nuclei characterized by high neutron excess is crucial for such verifications as well as for the {tau}-process nucleosynthesis scenario. Heavy neutron-rich nuclei, south-east of doubly-magic {sup 208}Pb, were always very difficult to produce and investigate. The nuclei like {sup 218}Po and {sup 214}Pb or {sup 210}Tl marked the border line of known nuclei from the beginning of the radioactivity era for over ninety years. To illustrate the difficulties, one can refer to the experiments employing the on-line mass separator technique. A spallation of heavy targets like {sup 232}Th and {sup 238}U by high-energy protons was proven as a source of heavy neutron-rich nuclei. The isotopes near and beyond doubly-magic {sup 208}Pb were produced too. However, such studies often suffered from an isobaric contamination of much more strongly produced and efficiently released elements like francium or radon and their decay products. A new experimental technique, based on the pulsed release element selective method recently developed at the PS Booster-ISOLDE at CERN [7,8,9] greatly reduces the contamination of these very short-lived {alpha}-emitters (Z {ge} 84) for the isobaric mass chains A=215 to A=218.

  2. Short Lived Climate Pollutants cause a Long Lived Effect on Sea-level Rise: Analyzing climate metrics for sea-level rise

    NASA Astrophysics Data System (ADS)

    Sterner, E.; Johansson, D. J.

    2013-12-01

    Climate change depends on the increase of several different atmospheric pollutants. While long term global warming will be determined mainly by carbon dioxide, warming in the next few decades will depend to a large extent on short lived climate pollutants (SLCP). Reducing emissions of SLCPs could contribute to lower the global mean surface temperature by 0.5 °C already by 2050 (Shindell et al. 2012). Furthermore, the warming effect of one of the most potent SLCPs, black carbon (BC), may have been underestimated in the past. Bond et al. (2013) presents a new best estimate of the total BC radiative forcing (RF) of 1.1 W/m2 (90 % uncertainty bounds of 0.17 to 2.1 W/m2) since the beginning of the industrial era. BC is however never emitted alone and cooling aerosols from the same sources offset a majority of this RF. In the wake of calls for mitigation of SLCPs it is important to study other aspects of the climate effect of SLCPs. One key impact of climate change is sea-level rise (SLR). In a recent study, the effect of SLCP mitigation scenarios on SLR is examined. Hu et al (2013) find a substantial effect on SLR from mitigating SLCPs sharply, reducing SLR by 22-42% by 2100. We choose a different approach focusing on emission pulses and analyse a metric based on sea level rise so as to further enlighten the SLR consequences of SLCPs. We want in particular to understand the time dynamics of SLR impacts caused by SLCPs compared to other greenhouse gases. The most commonly used physical based metrics are GWP and GTP. We propose and evaluate an additional metric: The global sea-level rise potential (GSP). The GSP is defined as the sea level rise after a time horizon caused by an emissions pulse of a forcer to the sea level rise after a time horizon caused by an emissions pulse of a CO2. GSP is evaluated and compared to GWP and GTP using a set of climate forcers chosen to cover the whole scale of atmospheric perturbation life times (BC, CH4, N2O, CO2 and SF6). The study

  3. The possibility to measure the magnetic moments of short-lived particles (charm and beauty baryons) at LHC and FCC energies using the phenomenon of spin rotation in crystals

    NASA Astrophysics Data System (ADS)

    Baryshevsky, V. G.

    2016-06-01

    The use of spin rotation effect in bent crystals for measuring the magnetic moment of short-lived particles in the range of LHC and FCC energies is considered. It is shown that the estimated number of produced baryons that are captured into a bent crystal grows as ∼γ 3 / 2 with increasing particle energy. Hence it may be concluded that the experimental measurement of magnetic moments of short-lived particles using the spin rotation effect is feasible at LHC and higher energies (for LHC energies, e.g., the running time required for measuring the magnetic moment of Λc+is 2 ÷ 16 hours).

  4. The possibility to measure the magnetic moments of short-lived particles (charm and beauty baryons) at LHC and FCC energies using the phenomenon of spin rotation in crystals

    NASA Astrophysics Data System (ADS)

    Baryshevsky, V. G.

    2016-06-01

    The use of spin rotation effect in bent crystals for measuring the magnetic moment of short-lived particles in the range of LHC and FCC energies is considered. It is shown that the estimated number of produced baryons that are captured into a bent crystal grows as ∼γ 3 / 2 with increasing particle energy. Hence it may be concluded that the experimental measurement of magnetic moments of short-lived particles using the spin rotation effect is feasible at LHC and higher energies (for LHC energies, e.g., the running time required for measuring the magnetic moment of Λc+ is 2 ÷ 16 hours).

  5. Composition and Trends of Short-Lived Trace Gases in the UT/LS over Europe Observed by the CARIBIC Aircraft

    NASA Astrophysics Data System (ADS)

    Baker, A. K.; Brenninkmeijer, C. A.; Oram, D. E.; O'Sullivan, D. A.; Slemr, F.; Schuck, T. J.

    2009-12-01

    The CARIBIC project (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container) involves the monthly deployment of an instrument container equipped to make atmospheric measurements from aboard a commercial airliner, and has operated since 2005 from aboard a Lufthansa Airbus 340-600 . Measurements from the container include in-situ trace gas and aerosol analyses and the collection of aerosol and whole air samples for post-flight laboratory analysis. Measurements made from the sampling flasks include greenhouse gas (GHG), halocarbon and nonmethane hydrocarbon (NMHC) analysis. CARIBIC flights originate in Frankfurt, Germany with routes to India, East Asia, South America, North America and Africa, and typical aircraft cruising altitudes of 10-12km allow for the monitoring of the upper troposphere/lower stratosphere (UT/LS) along these routes. Data collected during the aircraft’s departure from and return to Frankfurt provide a 4 year time series of near-monthly measurements of the composition of the UT/LS above Europe. Here we present a discussion of the composition of short-lived trace gases in the whole air samples collected above Europe during CARIBIC flights. Over 150 air samples were collected between May 2005 and July 2009, or about 4 samples per month. Of the whole air samples collected, about 45% showed influence by stratospheric air (i.e. very low values of GHG, NMHC and halocarbons, elevated O3, high potential vorticity). The remaining samples were representative of the upper troposphere; back trajectories for these samples indicate that a little over half were collected in air masses that had been in the boundary layer within the previous 8 days. The predominant source regions for these samples were the Gulf of Mexico and continental North America. Owing to their wide range of chemical lifetimes and the varying composition of emissions, short-lived trace gases transported to the UT/LS can be useful indicators of source

  6. An alternative approach to comparing long- and short-lived emissions in light of the 2&amp;deg;C global temperature limit

    NASA Astrophysics Data System (ADS)

    Smith, Stephen; Bowerman, Niel; Lowe, Jason; Huntingford, Chris; Frame, Dave; Allen, Myles; Gohar, Laila; Millar, Richard

    2014-05-01

    International climate policy has defined its goal in terms of limiting global average temperature, specifically to 2°C above pre-industrial levels. Emissions of several different greenhouse gases (GHGs) are currently aggregated and traded in terms of their carbon dioxide equivalent. The metric used for aggregating and trading is the 100-year Global Warming Potential (GWP100). Importantly though, the GWP100 does not measure temperature and so does clearly indicate the relative value of different emissions in the context of a global temperature limit. Recent developments in climate research have led to two different, potentially conflicting, perspectives on priorities in reducing emissions. First, a clear link has been demonstrated between cumulative emissions of carbon dioxide and peak temperature. This emphasises the need for carbon dioxide emissions to fall to near zero and provides a conceptually neat way to frame policy, but says little about the role of other GHGs. Second, other studies have shown that emissions of short-lived climate pollutants (SLCPs), many of which currently lie outside climate policy, have a substantial near-term effect on climate. It has been suggested that immediate SLCP reductions will therefore increase the chance of staying below 2°C and may even "buy time" for carbon dioxide reductions. This presentation summarises two recent papers which clarify the roles of SLCPs and long-lived GHGs in determining peak global temperature, and propose new emission metrics to reflect these. SLCP emissions reductions in a given decade have a significant impact on peak temperature only if carbon dioxide emissions are already falling. Immediate action on SLCPs might potentially "buy time" for adaptation by reducing near-term warming, but it does not buy time to delay reductions in carbon dioxide compared with delayed SLCP reductions. Peak temperature is ultimately constrained by cumulative emissions of several long-lived gases (including carbon dioxide

  7. Very short-lived bromomethanes measured by the CARIBIC observatory over the North Atlantic, Africa and South-East Asia during 2009-2013

    NASA Astrophysics Data System (ADS)

    Wisher, A.; Oram, D. E.; Laube, J. C.; Mills, G. P.; van Velthoven, P.; Zahn, A.; Brenninkmeijer, C. A. M.

    2013-11-01

    Short-lived organic brominated compounds make up a significant part (~20%) of the organic bromine budget in the atmosphere. Emissions of these compounds are highly variable and there are limited measurements, particularly in the extra-tropical upper troposphere/lower stratosphere and tropical troposphere. Measurements of five short-lived bromomethanes (VSLB) were made in air samples collected on the CARIBIC project aircraft over three flight routes; Germany to Venezuela/Columbia during 2009-2011, Germany to South Africa during 2010 and 2011 and Germany to Thailand/Kuala Lumpur, Malaysia during 2012 and 2013. In the tropical troposphere, as the most important entrance region to the stratosphere, we observe a total mean organic bromine derived from these compounds across all flights at 10-12 km altitude of 3.4 ± 1.5 ppt. Individual mean tropical tropospheric mixing ratios across all flights were 0.43, 0.74, 0.14, 0.23 and 0.11 ppt for CHBr3, CH2Br2, CHBr2Cl, CHBrCl2 and CH2BrCl respectively. The highest levels of VSLS-derived bromine (4.20 ± 0.56 ppt) were observed in flights between Bangkok and Kuala Lumpur indicating that the South China Sea is an important source region for these compounds. Across all routes, CHBr3 and CH2Br2 accounted for 34% (4.7-71) and 48% (14-73) respectively of total bromine derived from the analysed VSLB in the tropical mid-upper troposphere totalling 82% (54-89). In samples collected between Germany and Venezuela/Columbia, we find decreasing mean mixing ratios with increasing potential temperature in the extra-tropics. Tropical mean mixing ratios are higher than extra-tropical values between 340-350 K indicating that rapid uplift is important in determining mixing ratios in the lower tropical tropopause layer in the West Atlantic tropics. O3 was used as a tracer for stratospherically influenced air and we detect rapidly decreasing mixing ratios for all VSLB above ~100 ppb O3 corresponding to the extra-tropical tropopause layer.

  8. Increased Concentrations of Short-Lived Decay-Series Radionuclides in Groundwaters Underneath the Nopal I Uranium Deposit at Pena Blanca, Mexico

    NASA Astrophysics Data System (ADS)

    Luo, S.; Ku, T.; Todd, V.; Murrell, M. T.; Dinsmoor, J. C.

    2007-05-01

    The Nopal I uranium ore deposit at Pena Blanca, Mexico, located at > 200 meters above the groundwater table, provides an ideal natural analog for quantifying the effectiveness of geological barrier for isolation of radioactive waste nuclides from reaching the human environments through ground water transport. To fulfill such natural analog studies, three wells (PB1, PB2, and PB3 respectively) were drilled at the site from the land surface down to the saturated groundwater zone and ground waters were collected from each of these wells through large- volume sampling/in-situ Mn-filter filtration for analyses of short-lived uranium/thorium-series radionuclides. Our measurements from PB1 show that the groundwater standing in the hole has much lower 222Rn activity than the freshly pumped groundwater. From this change in 222Rn activity, we estimate the residence time of groundwater in PB1 to be about 20 days. Our measurements also show that the activities of short-lived radioisotopes of Th (234Th), Ra (228Ra, 224Ra, 223Ra), Rn (222Rn), Pb (210Pb), and Po (210Po) in PB1, PB2, and PB3 are all significantly higher than those from the other wells near the Nopal I site. These high activities provide evidence for the enrichment of long-lived U and Ra isotopes in the groundwater as well as in the associated adsorbed phases on the fractured aquifer rocks underneath the ore deposit. Such enrichment suggests a rapid dissolution of U and Ra isotopes from the uranium ore deposit in the vadose zone and the subsequent migration to the groundwater underneath. A reactive transport model can be established to characterize the in-situ transport of radionuclides at the site. The observed change of 222Rn activity at PB1 also suggests that the measured high radioactivityies in ground waters from the site isare not an artifact of drilling operations. However, further studies are needed to assess if or to what extent the radionuclide migration is affected by the previous mining activities at

  9. Very short-lived bromomethanes measured by the CARIBIC observatory over the North Atlantic, Africa and Southeast Asia during 2009-2013

    NASA Astrophysics Data System (ADS)

    Wisher, A.; Oram, D. E.; Laube, J. C.; Mills, G. P.; van Velthoven, P.; Zahn, A.; Brenninkmeijer, C. A. M.

    2014-04-01

    Short-lived organic brominated compounds make up a significant part of the organic bromine budget in the atmosphere. Emissions of these compounds are highly variable and there are limited measurements, particularly in the extra-tropical upper troposphere/lower stratosphere and tropical troposphere. Measurements of five very short-lived bromomethanes (VSLB) were made in air samples collected on the CARIBIC project aircraft over three flight routes; Germany to Venezuela/Columbia during 2009-2011, Germany to South Africa during 2010 and 2011 and Germany to Thailand/Kuala Lumpur, Malaysia during 2012 and 2013. In the tropical troposphere, as the most important entrance region to the stratosphere, we observe a total mean organic bromine derived from these compounds across all flights at 10-12 km altitude of 3.4 ± 1.5 ppt. Individual mean tropical tropospheric mixing ratios across all flights were 0.43, 0.74, 0.14, 0.23 and 0.11 ppt for CHBr3, CH2Br2, CHBr2Cl, CHBrCl2 and CH2BrCl respectively. The highest levels of VSLB-derived bromine (4.20 ± 0.56 ppt) were observed in flights between Bangkok and Kuala Lumpur indicating that the South China Sea is an important source region for these compounds. Across all routes, CHBr3 and CH2Br2 accounted for 34% (4.7-71) and 48% (14-73) respectively of total bromine derived from the analysed VSLB in the tropical mid-upper troposphere totalling 82% (54-89). In samples collected between Germany and Venezuela/Columbia, we find decreasing mean mixing ratios with increasing potential temperature in the extra-tropics. Tropical mean mixing ratios are higher than extra-tropical values between 340-350 K indicating that rapid uplift is important in determining mixing ratios in the lower tropical tropopause layer in the West Atlantic tropics. O3 was used as a tracer for stratospherically influenced air and we detect rapidly decreasing mixing ratios for all VSLB above ∼100 ppb O3 corresponding to the extra-tropical tropopause layer.

  10. Short-lived Supershear Rupture

    NASA Astrophysics Data System (ADS)

    Fukuyama, E.; Xu, S.; Yamashita, F.; Mizoguchi, K.; Takizawa, S.; Kawakata, H.

    2015-12-01

    Fukuyama and Olsen (2002) computed the supershear rupture initiation, propagation and termination process due to a passage of high stress drop area (called asperity) using a boundary integral equation method. They found that supershear rupture continued to propagate after the passage through high stress drop area but it died after a certain propagation distance, which depends on the elastic energy released at the high stress drop area. Here, we could reproduce a similar phenomenon in the laboratory. We conducted large-scale biaxial friction experiments using a pair of meter-scaled metagabbro rock specimens (VP=6.9km/s, VS=3.6km/s) at the National Research institute for Earth Science and Disaster Prevention (NIED). We observed several stick slip rupture events that initiated close to an asperity and immediately became supershear ruptures. But after propagating certain distance they died out and co-existing subshear ruptures became prominent. If we look into details, during the supershear rupture, we could see a sequence of rupture acceleration, its short rest and re-acceleration. This feature reminds us of a sequential breakage of small high stress patches as predicted by Fukuyama and Madariaga (2000). These observations might be interpreted under a concept of energy balance where the energy transmission from strain energy released by the asperity to fracture energy consumed at the crack tip was not instantaneously balanced in space. This could be related to the fact that earthquake rupture velocity is rather smooth reported from the finite fault analysis of large earthquakes with seismic waveforms. References Fukuyama, E. and R. Madariaga (2000) Dynamic propagation and interaction of a rupture front on a planar fault, PAGEOPH, 257, 1959-1979. Fukuyama, E. and K.B. Olsen (2002) A condition for super-shear rupture propagation in a heterogeneous stress field, PAGEOPH, 159, 2047-2056.

  11. Individual thyroid dose estimation for a case-control study of Chernobyl-related thyroid cancer among children of Belarus-part I: 131I, short-lived radioiodines (132I, 133I, 135I), and short-lived radiotelluriums (131MTe and 132Te).

    PubMed

    Gavrilin, Yuri; Khrouch, Valeri; Shinkarev, Sergey; Drozdovitch, Vladimir; Minenko, Victor; Shemiakina, Elena; Ulanovsky, Alexander; Bouville, André; Anspaugh, Lynn; Voillequé, Paul; Luckyanov, Nickolas

    2004-06-01

    Large amounts of radioiodines were released into the atmosphere during the accident at the Chernobyl nuclear power plant on 26 April 1986. In order to investigate whether the thyroid cancers observed among children in Belarus could have been caused by radiation exposures from the Chernobyl accident, a team of Belarusian, Russian, and American scientists conducted a case-control study to compare cases and controls according to estimated thyroid dose. The primary purpose of this paper is to present detailed information on the estimated thyroid doses, due to intakes of 131I, that were used in the case-control study. The range of the 131I thyroid doses among the 107 cases and the 214 controls was found to extend from 0.00002 to 4.3 Gy, with medians of approximately 0.2 Gy for the cases and 0.07 Gy for the controls. In addition, the thyroid doses resulting from the intakes of short-lived radioiodines (132I, 133I, and 135I) and radiotelluriums (131mTe and 132Te) were estimated and compared to the doses from 131I. The ratios of the estimated thyroid doses from the short-lived radionuclides and from I for the cases and the controls range from 0.003 to 0.1, with median values of approximately 0.02 for both cases and controls. PMID:15167120

  12. The origin and disappearance of the late Pleistocene-early Holocene short-lived coastal wetlands along the Carmel coast, Israel

    NASA Astrophysics Data System (ADS)

    Sivan, Dorit; Greenbaum, Noam; Cohen-Seffer, Ronit; Sisma-Ventura, Guy; Almogi-Labin, Ahuva

    The formation of short-lived backswamps along the Carmel coast of Israel coincides with the rapid global sea-level rise during the late Pleistocene-early Holocene transition. The current study shows that the wetland phenomena originated around 10,000 yr ago and dried up shortly before the local Pre-Pottery Neolithic humans settled on the wetland dark clay sediments 9430 cal yr BP. Palaeontological and stable-isotope data were used in this study to elucidate previously published sedimentological reconstruction obtained from a core drilled into the western trough of the Carmel coastal plain. The water body contained typical brackish calcareous fauna, with variable numerical abundance and low species richness of ostracods and foraminifera. The δ 18O and δ 13C of the ostracod Cyprideis torosa show close similarity to the present Pleistocene coastal aquifer isotopic values. This study therefore concludes that the wetlands were shallow-water bodies fed by groundwater, with no evidence of sea-water mixing. It seems that they developed as the result of high groundwater levels, transportation of sediments landward, and deposition of sand bars at the paleo-river mouths. It is still not fully understood why these wetlands deteriorated abruptly and disappeared within less than 1000 yr.

  13. Kinetics and Mechanism of the Chlorite-Periodate System: Formation of a Short-Lived Key Intermediate OClOIO3 and Its Subsequent Reactions.

    PubMed

    Baranyi, Nóra; Csekő, György; Valkai, László; Xu, Li; Horváth, Attila K

    2016-03-01

    The chlorite-periodate reaction has been studied spectrophotometrically in acidic medium at 25.0 ± 0.1 °C, monitoring the absorbance at 400 nm in acetate/acetic acid buffer at constant ionic strength (I = 0.5 M). We have shown that periodate was exclusively reduced to iodate, but chlorite ion was oxidized to chlorate and chlorine dioxide via branching pathways. The stoichiometry of the reaction can be described as a linear combination of two limiting stoichiometries under our experimental conditions. Detailed initial rate studies have clearly revealed that the formal kinetic orders of hydrogen ion, chlorite ion, and periodate ion are all strictly one, establishing an empirical rate law to be d[ClO2]/dt = kobs[ClO2(-)][IO4(-)][H(+)], where the apparent rate coefficient (kobs) was found to be 70 ± 13 M(-2) s(-1). On the basis of the experiments, a simple four-step kinetic model with three fitted kinetic parameters is proposed by nonlinear parameter estimation. The reaction was found to proceed via a parallel oxygen transfer reaction leading to the exclusive formation of chlorate and iodate as well as via the formation of a short-lived key intermediate OClOIO3 followed by its further transformations by a sequence of branching pathways. PMID:26849795

  14. Tropospheric ozone and its precursors from the urban to the global scale from air quality to short-lived climate forcer

    NASA Astrophysics Data System (ADS)

    Monks, P. S.; Archibald, A. T.; Colette, A.; Cooper, O.; Coyle, M.; Derwent, R.; Fowler, D.; Granier, C.; Law, K. S.; Stevenson, D. S.; Tarasova, O.; Thouret, V.; von Schneidemesser, E.; Sommariva, R.; Wild, O.; Williams, M. L.

    2014-12-01

    Ozone holds a certain fascination in atmospheric science. It is ubiquitous in the atmosphere, central to tropospheric oxidation chemistry, yet harmful to human and ecosystem health as well as being an important greenhouse gas. It is not emitted into the atmosphere but is a by-product of the very oxidation chemistry it largely initiates. Much effort is focussed on the reduction of surface levels of ozone owing to its health impacts but recent efforts to achieve reductions in exposure at a country scale have proved difficult to achieve due to increases in background ozone at the zonal hemispheric scale. There is also a growing realisation that the role of ozone as a short-lived climate pollutant could be important in integrated air quality climate-change mitigation. This review examines current understanding of the processes regulating tropospheric ozone at global to local scales from both measurements and models. It takes the view that knowledge across the scales is important for dealing with air quality and climate change in a synergistic manner.

  15. Tropospheric ozone and its precursors from the urban to the global scale from air quality to short-lived climate forcer

    NASA Astrophysics Data System (ADS)

    Monks, P. S.; Archibald, A. T.; Colette, A.; Cooper, O.; Coyle, M.; Derwent, R.; Fowler, D.; Granier, C.; Law, K. S.; Mills, G. E.; Stevenson, D. S.; Tarasova, O.; Thouret, V.; von Schneidemesser, E.; Sommariva, R.; Wild, O.; Williams, M. L.

    2015-08-01

    Ozone holds a certain fascination in atmospheric science. It is ubiquitous in the atmosphere, central to tropospheric oxidation chemistry, yet harmful to human and ecosystem health as well as being an important greenhouse gas. It is not emitted into the atmosphere but is a byproduct of the very oxidation chemistry it largely initiates. Much effort is focused on the reduction of surface levels of ozone owing to its health and vegetation impacts, but recent efforts to achieve reductions in exposure at a country scale have proved difficult to achieve owing to increases in background ozone at the zonal hemispheric scale. There is also a growing realisation that the role of ozone as a short-lived climate pollutant could be important in integrated air quality climate change mitigation. This review examines current understanding of the processes regulating tropospheric ozone at global to local scales from both measurements and models. It takes the view that knowledge across the scales is important for dealing with air quality and climate change in a synergistic manner. The review shows that there remain a number of clear challenges for ozone such as explaining surface trends, incorporating new chemical understanding, ozone-climate coupling, and a better assessment of impacts. There is a clear and present need to treat ozone across the range of scales, a transboundary issue, but with an emphasis on the hemispheric scales. New observational opportunities are offered both by satellites and small sensors that bridge the scales.

  16. Comparison of short-lived high-LET alpha-emitting radionuclides lead-212 and bismuth-212 to low-LET X-rays on ovarian carcinoma.

    PubMed

    Rotmensch, J; Atcher, R W; Hines, J; Toohill, M; Herbst, A L

    1989-12-01

    We are investigating the potential use of short-lived alpha-emitting radionuclides for the treatment of ovarian carcinoma. These radionuclides transfer dense high ionizing linear energy (high LET) over a short path length without dependence upon cellular oxygen. The alpha-emitting radionuclides chosen were lead-212 and bismuth-212 which are readily available. The radiosensitivities of two ovarian carcinoma cell lines (OVC-1 and OVC-2) was greater with 212Pb and 212Bi than with X-ray therapy. D0, inversely related to the radiosensitivity, was 155 and 240 rads for OVC-1 and OVC-2, respectively. With 212Pb or 212Bi, the slope of the survival curves was steeper. The D0 was 75 and 70 rads after 212Pb and 85 and 95 rads after 212Bi treatment for OVC-1 and OVC-2, respectively. The relative biological effectiveness with alpha irradiation was two to four times greater than with X rays. Unlike low-LET irradiation (i.e., X rays and gamma emitters) the cells had no ability to accumulate or repair sublethal damage. From these experiments it is concluded that a greater therapeutic advantage may be gained with alpha-emitting radionuclides than X rays. Further development of these nuclides may provide for a new form of therapy. PMID:2599463

  17. Some observations on the concentrations of short-lived decay products of radon and thoron in the monsoon rains of Bombay, India

    NASA Astrophysics Data System (ADS)

    Rangarajan, C.; Eapen, C. D.

    1985-08-01

    The concentrations of radon decay products 214Pb(RaB) and 214Bi(RaC) and thoron daughter 212Pb(ThB) have been measured in rainfall at Bombay. The presence of short-lived 218Po(RaA) is indicated in a few samples. The levels of 214Pb varied from 300 to 7000 pCi (11-260 Bq) per liter, while the activity ratios of 214Bi/214Pb are in the range of 0.5-1.5. From these values of the ratios a cloud drop lifetime, from nucleation to deposition, of 20-60 min is estimated. The concentrations of 212Pb varied from 2 to 30 pCi (0.075-1.1 Bq) per liter. The levels of radon and thoron daughter products are lower in Bombay summer rainfall compared with other areas due to their reduced concentrations in the maritime monsoon winds. Approximate estimates of scavenging ratios based on the surface air concentrations are 85±65 (1 standard deviation) and 30±20 (1 standard deviation) for radon and thoron daughters, respectively.

  18. Combining radon, short-lived radium isotopes and hydrodynamic modeling to assess submarine groundwater discharge from an anthropized semiarid watershed to a Mediterranean lagoon (Mar Menor, SE Spain)

    NASA Astrophysics Data System (ADS)

    Baudron, Paul; Cockenpot, Sabine; Lopez-Castejon, Francisco; Radakovitch, Olivier; Gilabert, Javier; Mayer, Adriano; Garcia-Arostegui, José Luis; Martinez-Vicente, David; Leduc, Christian; Claude, Christelle

    2015-06-01

    In highly anthropized watersheds, surface water tributaries may carry unexpected high quantities of radon and radium to coastal lagoons. Investigating submarine groundwater discharge (SGD) with radionuclide tracers is therefore a complex task. In order to quantify SGD and decipher the influence of the different water sources, we combined a radon (222Rn) and short-lived radium (223Ra, 224Ra) survey with the hydrodynamic modeling of a lagoon. We applied it to the Mar Menor lagoon (SE Spain) where surface water tributaries and undocumented emissaries carry water from groundwater drainage and brines from groundwater desalinization. We identified the areas of influence of the plume of radionuclides from the river, located major areas of SGD and proposed a location for two submarine emissaries. Porewater, i.e. interstitial water from underlying sediments, was found to be the most representative SGD end member, compared to continental groundwater collected from piezometers. Mass balances in winter and summer seasons provided yearly SGD fluxes of water of 0.4-2.2 ṡ 108 m3/y (222Rn), 4.4-19.0 ṡ 108 m3/y (224Ra) and 1.3 ṡ 108 m3/y (223Ra, measured in winter only). Tidal pumping was identified as a main driver for recirculated saline groundwater, while fresh submarine groundwater discharge from the aquifer ranged between 2% and 23% of total SGD.

  19. Triggering Collapse of the Presolar Dense Cloud Core and Injecting Short-lived Radioisotopes with a Shock Wave. IV. Effects of Rotational Axis Orientation

    NASA Astrophysics Data System (ADS)

    Boss, Alan P.; Keiser, Sandra A.

    2015-08-01

    Both astronomical observations of the interaction of Type II supernova remnants (SNRs) with dense interstellar clouds as well as cosmochemical studies of the abundances of daughter products of short-lived radioisotopes (SLRIs) formed by supernova nucleosynthesis support the hypothesis that the Solar System's SLRIs may have been derived from a supernova. This paper continues a series devoted to examining whether or not such a shock wave could have triggered the dynamical collapse of a dense, presolar cloud core and simultaneously injected sufficient abundances of SLRIs to explain the cosmochemical evidence. Here, we examine the effects of shock waves striking clouds whose spin axes are oriented perpendicular, rather than parallel, to the direction of propagation of the shock front. The models start with 2.2 {M}⊙ cloud cores and shock speeds of 20 or 40 km s-1. Central protostars and protoplanetary disks form in all models, although with their disk spin axes aligned somewhat randomly. The disks derive most of their angular momentum not from the initial cloud rotation, but from the Rayleigh-Taylor fingers that also inject shock wave SLRIs. Injection efficiencies, fi, the fraction of the incident shock wave material injected into the collapsing cloud core, are ˜0.04-0.1 in these models, similar to when the rotation axis is parallel to the shock propagation direction. Evidently, altering the rotation axis orientation has only a minor effect on the outcome, strengthening the case for this scenario as an explanation for the Solar System's SLRIs.

  20. Diurnal variation climatology of short-lived at atmospheric compositions (ClO, BrO, HO2 and HOCl) derived from SMILES NICT data

    NASA Astrophysics Data System (ADS)

    Kreyling, Daniel; Sagawa, Hideo; Kasai, Yasuko

    2013-04-01

    We present a diurnal variation climatology for short-lived at atmospheric compositions, such as ClO, BrO, HO2 and HOCl, as well as for longer life time species, like O3 and HCl from observations of unprecedented sensitivity with the Superconducting SubMIllimeter wave Limb-Emission Sounder (SMILES), which is installed on the Japanese Experiment Module (JEM) at the International Space Station (ISS). With its non sun synchronous orbit, SMILES measurements comprise observations at all local times. The target altitude range is between lower stratosphere and mesopause. Differences in diurnal variation chemistry of strato-, and mesospheric BrO and ClO of the diurnal climatology are presented. The data employed is produced by the SMILES level 2 retrieval algorithm version 2.1.5 at the National Institute of Information and Communications Technology (NICT). The SMILES climatology data sets are available via the SMILES data distribution homepage in NICT at https://smiles-p6.nict.go.jp/products/research_latitude-longitude.jsf

  1. Climate impacts of short-lived climate forcers versus CO2 from biodiesel: a case of the EU on-road sector.

    PubMed

    Lund, Marianne T; Berntsen, Terje K; Fuglestvedt, Jan S

    2014-12-16

    Biofuels are proposed to play an important role in several mitigation strategies to meet future CO2 emission targets for the transport sector but remain controversial due to significant uncertainties in net impacts on environment, society, and climate. A switch to biofuels can also affect short-lived climate forcers (SLCFs), which provide significant contributions to the net climate impact of transportation. We quantify the radiative forcing (RF) and global-mean temperature response over time to EU on-road fossil diesel SLCFs and the impact of 20% (B20) and 100% (B100) replacement of fossil diesel by biodiesel. SLCFs are compared to impacts of on-road CO2 using different approaches from existing literature to account for biodiesel CO2. Given the best estimates for changes in emissions when replacing fossil diesel with biodiesel, the net positive RF from EU on-road fossil diesel SLCFs of 3.4 mW/m(2) is reduced by 15% and 80% in B20 and B100, respectively. Over time the warming of SLCFs is likely small compared to biodiesel CO2 impacts. However, SLCFs may be relatively more important for the total warming than in the fossil fuel case if biodiesel from feedstock with very short rotation periods and low land-use-change impacts replaces a high fraction of fossil diesel. PMID:25405926

  2. Effective Strategy for Conformer-Selective Detection of Short-Lived Excited State Species: Application to the IR Spectroscopy of the N1H Keto Tautomer of Guanine.

    PubMed

    Asami, Hiroya; Tokugawa, Munefumi; Masaki, Yoshiaki; Ishiuchi, Shun-Ichi; Gloaguen, Eric; Seio, Kohji; Saigusa, Hiroyuki; Fujii, Masaaki; Sekine, Mitsuo; Mons, Michel

    2016-04-14

    The ultrafast deactivation processes in the excited state of biomolecules, such as the most stable tautomers of guanine, forbid any state-of-the-art gas phase spectroscopic studies on these species with nanosecond lasers. This drawback can be overcome by grafting a chromophore having a long-lived excited state to the molecule of interest, allowing thus a mass-selective detection by nanosecond R2PI and therefore double resonance IR/UV conformer-selective spectroscopic studies. The principle is presently demonstrated on the keto form of a modified 9-methylguanine, for which the IR/UV double resonance spectrum in the C═O stretch region, reported for the first time, provides evidence for extensive vibrational couplings within the guanine moiety. Such a successful strategy opens up a route to mass-selective IR/UV spectroscopic investigations on molecules exhibiting natural chromophores having ultrashort-lived excited states, such as DNA bases, their complexes as well as peptides containing short-lived aromatic residues. PMID:26990184

  3. Significance of Nain-Baft ophiolitic belt (Iran): Short-lived, transtensional Cretaceous back-arc oceanic basins over the Tethyan subduction zone

    NASA Astrophysics Data System (ADS)

    Moghadam, Hadi Shafaii; Whitechurch, Hubert; Rahgoshay, Mohamad; Monsef, Iman

    2009-12-01

    Four dismembered massifs belonging to the Nain-Baft ophiolitic belt (Central Iran) stretch in a NW-SE direction parallel to the fossil active margin of the Iranian Continental Block (Sanandaj-Sirjan Zone). They are separated by huge transcurrent faults. The Nain, Dehshir, Shahr-e-Babak and Baft massifs are composed of associated slices of harzburgites, small bodies of gabbros and dike swarm complexes, accompanied by various extrusives from basaltic-andesitic lava flows and breccias to dacites and rhyolites. Trace element geochemistry of these lavas displays calc-alkaline and arc-tholeiite signatures, suggesting a back-arc origin for these ophiolites. This is in accordance with the position of these massifs, to the North of the Mesozoic Magmatic Arc crosscutting the Sanadaj-Sirjan Zone. Conventional K-Ar datings on amphibole within amphibolite and gabbros deliver ages between 93 Ma and 67 Ma. These ages are in good agreement with the stratigraphic age of the conformably Cenomanian to Maastrichtian sedimentary cover of the extrusives. The closure of these back-arc basins occurred in the Middle Paleocene as testified by the presence of neritic limestones, sealing all the tectonic contacts. The general geological setting of the Nain-Baft belt suggests that these massifs generated in a transtensional small back-arc basins separated by transcurrent faults. These short-lived transtensional basins result from the oblique subduction of the Tethyan Ocean under the Iranian Continental Block.

  4. Coulomb excitation studies of shape coexistence in atomic nuclei

    NASA Astrophysics Data System (ADS)

    Görgen, Andreas; Korten, Wolfram

    2016-02-01

    Low-energy Coulomb excitation provides a well-understood means of exciting atomic nuclei and allows measuring electromagnetic moments that can be directly related to the nuclear shape. The availability of radioactive ion beams (RIBs) at energies near the Coulomb barrier has made it possible to study shape coexistence in a variety of short-lived exotic nuclei. This review presents a short overview of the methods related to multi-step Coulomb excitation experiments, followed by a discussion of several examples. The focus is on two mass regions where recent Coulomb excitation experiments have contributed to the quantitative understanding of shape coexistence: nuclei with mass A≈ 70 near the N = Z line and nuclei with A ≈ 100 near neutron number N = 60. Experimental results are summarized and their significance for understanding shape coexistence is discussed. Experimental observables such as quadrupole moments and electromagnetic transition strengths represent furthermore important benchmarks for advancing theoretical nuclear structure models. With several new RIB facilities planned and under construction, Coulomb excitation will remain to be an important tool to extend the studies of nuclear shapes toward more exotic systems, and to obtain a more comprehensive and quantitative understanding of shape coexistence.

  5. Studies of pear-shaped nuclei using accelerated radioactive beams.

    PubMed

    Gaffney, L P; Butler, P A; Scheck, M; Hayes, A B; Wenander, F; Albers, M; Bastin, B; Bauer, C; Blazhev, A; Bönig, S; Bree, N; Cederkäll, J; Chupp, T; Cline, D; Cocolios, T E; Davinson, T; De Witte, H; Diriken, J; Grahn, T; Herzan, A; Huyse, M; Jenkins, D G; Joss, D T; Kesteloot, N; Konki, J; Kowalczyk, M; Kröll, Th; Kwan, E; Lutter, R; Moschner, K; Napiorkowski, P; Pakarinen, J; Pfeiffer, M; Radeck, D; Reiter, P; Reynders, K; Rigby, S V; Robledo, L M; Rudigier, M; Sambi, S; Seidlitz, M; Siebeck, B; Stora, T; Thoele, P; Van Duppen, P; Vermeulen, M J; von Schmid, M; Voulot, D; Warr, N; Wimmer, K; Wrzosek-Lipska, K; Wu, C Y; Zielinska, M

    2013-05-01

    There is strong circumstantial evidence that certain heavy, unstable atomic nuclei are 'octupole deformed', that is, distorted into a pear shape. This contrasts with the more prevalent rugby-ball shape of nuclei with reflection-symmetric, quadrupole deformations. The elusive octupole deformed nuclei are of importance for nuclear structure theory, and also in searches for physics beyond the standard model; any measurable electric-dipole moment (a signature of the latter) is expected to be amplified in such nuclei. Here we determine electric octupole transition strengths (a direct measure of octupole correlations) for short-lived isotopes of radon and radium. Coulomb excitation experiments were performed using accelerated beams of heavy, radioactive ions. Our data on (220)Rn and (224)Ra show clear evidence for stronger octupole deformation in the latter. The results enable discrimination between differing theoretical approaches to octupole correlations, and help to constrain suitable candidates for experimental studies of atomic electric-dipole moments that might reveal extensions to the standard model. PMID:23657348

  6. The influence of s states near threshold on the structure of light nuclei

    NASA Astrophysics Data System (ADS)

    Hoffman, Calem

    2015-10-01

    A recent work identified the role of neutron s states, and their proximity to the neutron separation threshold, on the ordering of the 1s1 / 2 and 0d5 / 2 single-particle levels in light nuclei. A simple Woods-Saxon potential was used to reproduce the systematic data available for these two levels with great success by accounting for the s state binding energy. This talk will explore other noticeable trends in light nuclei involving neutron s states and utilizing simple potential models determine the role binding energy plays. The trends and calculations will aim to provide descriptions of data and predictions of yet to be found two-particle two-hole excited states in N = 8 and 10 nuclei ranging from Z = 4-9, as well as the energies of mirror states in neutron deficient Al and Na isotopes. Results will be compared with state-of-the-art calculations. Possible future measurements capable of probing these predictions will be discussed as well. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract Number DE-AC02-06CH11357.

  7. Spectroscopy of Mirror Nuclei in the Upper-fp Shell Using GRETINA

    NASA Astrophysics Data System (ADS)

    Clark, Roderick; Henry, Thomas; Bentley, Michael; E11025 Gretina@Msu Collaboration

    2013-10-01

    Isospin symmetry breaking in nuclei of the upper-fp shell has been investigated in a recent experiment at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). A 78Kr primary beam (with energy 150 MeV.A) was fragmented on a Be target to produce a cocktail of secondary beams, including 66As, 65Ge, and 64Ga, which were selected with the A1900 separator. These secondary beams were in turn fragmented at the target position of S800 magnetic spectrograph, which was used to identify neutron-deficient reaction products including 62,63Ga, 63Ge, and 65As. Gamma-rays emitted from excited states in these nuclei were detected with GRETINA, which comprises 28 highly-segmented, tapered hexagonal, close-packed HPGe and is a first generation gamma-ray tracking array. Many new states and transitions have been identified in these nuclei of the upper-fp shell, including a candidate for the T = 1 2+ state in 62Ga. Preliminary results from the analysis of this data will be presented and the implications for our understanding of isospin-symmetry breaking effects will be discussed. This work supported in part by the United States Department of Energy under grant no. DE-AC02-05CH11231 (LBNL).

  8. Decay studies of neutron deficient nuclei near the Z =64 subshell: sup 142 Dy, sup 140,142 Tb, sup 140,142 Gd, sup 140,142 Eu, sup 142 Sm, and

    SciTech Connect

    Firestone, R.B.; Gilat, J.; Nitschke, J.M.; Wilmarth, P.A.; Vierinen, K.S. )

    1991-03-01

    The electron-capture and {beta}{sup +}-decay branchings (EC/{beta}{sup +}) and delayed proton decays of {ital A}=142 isotopes with 61{le}{ital Z}{le}66 and {ital A}=140 isotopes with 63{le}{ital Z}{le}65 were investigated with the OASIS facility on-line at the Lawrence Berkeley Laboratory SuperHILAC. Electron capture and positron-decay emission probabilities have been determined for {sup 142}Pm and {sup 142}Sm decays, and extensive decay schemes have been constructed for {sup 142}Eu{sup {ital g}}(2.34{plus minus}0.12 s), {sup 142}Gd(70.2{plus minus}0.6 s), {sup 140}Eu(1.51{plus minus}0.02 s), and {sup 140}Gd(15.8{plus minus}0.4 s). Decay schemes for the new isotopes {sup 142}Tb{sup {ital g}}(597{plus minus}17 ms), {sup 142}Tb{sup {ital m}}(303{plus minus}17 ms), {sup 142}Dy(2.3{plus minus}0.3 s), {sup 140}Eu{sup {ital m}}(125{plus minus}2 ms), and {sup 140}Tb(2.4{plus minus}0.2 s) are also presented. We have assigned {gamma} rays to these isotopes on the basis of {gamma}{gamma} and {ital x}{gamma} coincidences, and from half-life determinations. Electron-capture and {beta}{sup +}-decay branchings were measured for each decay, and {beta}-delayed proton branchings were determined for {sup 142}Dy, {sup 142}Tb, and {sup 140}Tb decays. {ital Q}{sub EC} values, derived from the measured EC/{beta}{sup +} branchings and the level schemes are compared with those from the Wapstra and Audi mass evaluation and the Liran and Zeldes mass calculation. The systematics of the {ital N}=77 isomer decays are discussed, and the intense 0{sup +}{r arrow}1{sup +} and 1{sup +}{r arrow}0{sup +} ground-state beta decays are compared with shell-model predictions for simple spin-flip transitions.

  9. Decay studies of neutron deficient nuclei near the Z=64 subshell: 142Dy, 140,142Tb, 140,142Gd, 140,142Eu, 142Sm, and 142Pm

    NASA Astrophysics Data System (ADS)

    Firestone, R. B.; Gilat, J.; Nitschke, J. M.; Wilmarth, P. A.; Vierinen, K. S.

    1991-03-01

    The electron-capture and β+-decay branchings (EC/β+) and delayed proton decays of A=142 isotopes with 61<=Z<=66 and A=140 isotopes with 63<=Z<=65 were investigated with the OASIS facility on-line at the Lawrence Berkeley Laboratory SuperHILAC. Electron capture and positron-decay emission probabilities have been determined for 142Pm and 142Sm decays, and extensive decay schemes have been constructed for 142Eug(2.34+/-0.12 s), 142Gd(70.2+/-0.6 s), 140Eu(1.51+/-0.02 s), and 140Gd(15.8+/-0.4 s). Decay schemes for the new isotopes 142Tbg(597+/-17 ms), 142Tbm(303+/-17 ms), 142Dy(2.3+/-0.3 s), 140Eum(125+/-2 ms), and 140Tb(2.4+/-0.2 s) are also presented. We have assigned γ rays to these isotopes on the basis of γγ and xγ coincidences, and from half-life determinations. Electron-capture and β+-decay branchings were measured for each decay, and β-delayed proton branchings were determined for 142Dy, 142Tb, and 140Tb decays. QEC values, derived from the measured EC/β+ branchings and the level schemes are compared with those from the Wapstra and Audi mass evaluation and the Liran and Zeldes mass calculation. The systematics of the N=77 isomer decays are discussed, and the intense 0+-->1+ and 1+-->0+ ground-state beta decays are compared with shell-model predictions for simple spin-flip transitions.

  10. Chronic Parasitic Infection Maintains High Frequencies of Short-Lived Ly6C+CD4+ Effector T Cells That Are Required for Protection against Re-infection

    PubMed Central

    Peters, Nathan C.; Pagán, Antonio J.; Lawyer, Phillip G.; Hand, Timothy W.; Henrique Roma, Eric; Stamper, Lisa W.; Romano, Audrey; Sacks, David L.

    2014-01-01

    In contrast to the ability of long-lived CD8+ memory T cells to mediate protection against systemic viral infections, the relationship between CD4+ T cell memory and acquired resistance against infectious pathogens remains poorly defined. This is especially true for T helper 1 (Th1) concomitant immunity, in which protection against reinfection coincides with a persisting primary infection. In these situations, pre-existing effector CD4 T cells generated by ongoing chronic infection, not memory cells, may be essential for protection against reinfection. We present a systematic study of the tissue homing properties, functionality, and life span of subsets of memory and effector CD4 T cells activated in the setting of chronic Leishmania major infection in resistant C57Bl/6 mice. We found that pre-existing, CD44+CD62L−T-bet+Ly6C+ effector (TEFF) cells that are short-lived in the absence of infection and are not derived from memory cells reactivated by secondary challenge, mediate concomitant immunity. Upon adoptive transfer and challenge, non-dividing Ly6C+ TEFF cells preferentially homed to the skin, released IFN-γ, and conferred protection as compared to CD44+CD62L−Ly6C− effector memory or CD44+CD62L+Ly6C− central memory cells. During chronic infection, Ly6C+ TEFF cells were maintained at high frequencies via reactivation of TCM and the TEFF themselves. The lack of effective vaccines for many chronic diseases may be because protection against infectious challenge requires the maintenance of pre-existing TEFF cells, and is therefore not amenable to conventional, memory inducing, vaccination strategies. PMID:25473946

  11. RNA-seq of the aging brain in the short-lived fish N. furzeri - conserved pathways and novel genes associated with neurogenesis.

    PubMed

    Baumgart, Mario; Groth, Marco; Priebe, Steffen; Savino, Aurora; Testa, Giovanna; Dix, Andreas; Ripa, Roberto; Spallotta, Francesco; Gaetano, Carlo; Ori, Michela; Terzibasi Tozzini, Eva; Guthke, Reinhard; Platzer, Matthias; Cellerino, Alessandro

    2014-12-01

    The brains of teleost fish show extensive adult neurogenesis and neuronal regeneration. The patterns of gene regulation during fish brain aging are unknown. The short-lived teleost fish Nothobranchius furzeri shows markers of brain aging including reduced learning performances, gliosis, and reduced adult neurogenesis. We used RNA-seq to quantify genome-wide transcript regulation and sampled five different time points to characterize whole-genome transcript regulation during brain aging of N. furzeri. Comparison with human datasets revealed conserved up-regulation of ribosome, lysosome, and complement activation and conserved down-regulation of synapse, mitochondrion, proteasome, and spliceosome. Down-regulated genes differ in their temporal profiles: neurogenesis and extracellular matrix genes showed rapid decay, synaptic and axonal genes a progressive decay. A substantial proportion of differentially expressed genes (~40%) showed inversion of their temporal profiles in the last time point: spliceosome and proteasome showed initial down-regulation and stress-response genes initial up-regulation. Extensive regulation was detected for chromatin remodelers of the DNMT and CBX families as well as members of the polycomb complex and was mirrored by an up-regulation of the H3K27me3 epigenetic mark. Network analysis showed extensive coregulation of cell cycle/DNA synthesis genes with the uncharacterized zinc-finger protein ZNF367 as central hub. In situ hybridization showed that ZNF367 is expressed in neuronal stem cell niches of both embryonic zebrafish and adult N. furzeri. Other genes down-regulated with age, not previously associated with adult neurogenesis and with similar patterns of expression are AGR2, DNMT3A, KRCP, MEX3A, SCML4, and CBX1. CBX7, on the other hand, was up-regulated with age. PMID:25059688

  12. Resonant coherent excitation of Mg sup 11+ : Electronic collisions of state specified short-lived excited states in a crystal channel

    SciTech Connect

    Datz, S.; Dittner, P.F.; Gomez del Campo, J.; Krause, H.F.; Rosseel, T.M.; Vane, C.R. ); Iwata, I.; Komaki, I.; Kimura, M.; Yamazaki, Y. ); Fujimoto, F.; Honda, F. )

    1990-01-01

    Hydrogenic ions passing through axial and planar channels can be excited from n = 1 to n = 2 when the frequency of perturbation by the atoms in the crystal spaced a distance d apart comes into resonance with the spacing between eigenstates i and j {Delta}E{sub ij} = hK(v{sub i}/d) where K is a harmonic 1,2,3{hor ellipsis} of the (v{sub i}/d) frequency. The degeneracy in the n = 2 levels is removed; first by the assymetry in the crystal field and second by Stark mixing of 2s with 2p{sub x} which is caused by the wake field. Thus, the resonant frequency, and hence velocity, for excitation to 2p{sub x,y} is different than that for 2p{sub x} and they can be excited selectively. In the present work we used Mg{sup 11+}, where the n = 2 ionization cross section is small enough to permit escape of some of the excited ions from the crystal without being ionized by subsequent collisions and with the subsequent emission of radiation. Since we can excite different orientations of the ion selectively by varying the velocity we can measure the separate ionization cross sections for these states by determining the yields of totally stripped ions compared to those which emit a Ly {alpha} x-ray. A comparison of the two channels shows that the probability of escape from the crystal without ionizations is greater for ions in the 2p{sub x} state than those in the 2p{sub x,y} state. These RCE data and are presented as proof of principal for experiments which measure electron bombardment ionization cross sections for short lived excited states with specific polarization.

  13. Time-series variations of the short-lived Ra in coastal waters: implying input of SGD to the coastal zone of Da-Chia River, Taichung, Taiwan

    NASA Astrophysics Data System (ADS)

    Hsu, Feng-Hsin; Su, Chih-Chieh; Lin, In-Tain; Huh, Chih-An

    2015-04-01

    Submarine groundwater discharge (SGD) has been recognized as an important pathway for materials exchanging between land and sea. Input of SGD carries the associated nutrients, trace metals, and inorganic carbon that may makes great impacts on ecosystem in the coastal zone. Due to the variability of SGD magnitude, it is difficult to estimate the flux of those associated materials around the world. Even in the same area, SGD magnitude also varies in response to tide fluctuation and seasonal change on hydraulic gradient. Thus, long-term investigation is in need. In Taiwan, the SGD study is rare and the intrusion of seawater in the coastal aquifer is emphasized in previous studies. According to the information from Hydrogeological Data Bank (Central Geological Survey, MOEA), some areas still show potentiality of SGD. Here, we report the preliminary investigation result of SGD at Gaomei Wildlife Conservation Area which located at the south of the Da-Chia River mouth. This study area is characterized by a great tidal rang and a shallow aquifer with high groundwater recharge rate. Time-series measurement of the short-lived Ra in surface water was done in both dry and wet seasons at a tidal flat site and shows different trends of excess Ra-224 between dry and wet seasons. High excess Ra-224 activities (>20 dpm/100L) occurred at high tide in dry season but at low tide in wet season. The plot of salinity versus excess Ra-224, showing non-conservative curve, suggests that high excess Ra-224 activities derive from desorption in dry season but from SGD input in wet season.

  14. Dating the Laschamp Excursion: Why Speleothems are Valuable Tools for Constraining the Timing and Duration of Short-Lived Geomagnetic Events

    NASA Astrophysics Data System (ADS)

    Lascu, I.; Feinberg, J. M.; Dorale, J. A.; Cheng, H.; Edwards, R. L.

    2015-12-01

    Short-lived geomagnetic events are reflections of geodynamo behavior at small length scales. A rigorous documentation of the anatomy, timing, duration, and frequency of centennial-to-millennial scale geomagnetic events can be invaluable for theoretical and numerical geodynamo models, and for the understanding the finer dynamics of the Earth's core. A critical ingredient for characterizing such geomagnetic instabilities are tightly constrained age models that enable high-resolution magnetostratigraphies. Here we focus on a North American speleothem geomagnetic record of the Laschamp excursion, which was the first geomagnetic excursion recognized and described in the paleomagnetic record, and remains the most studied event of its kind. The geological significance of the Laschamp lies chiefly in the fact that it constitutes a global time-synchronous geochronological marker. The Laschamp excursion occurred around the time of the demise of Homo neanderthalensis, in conjunction with high-amplitude, rapid climatic oscillations leading into the Last Glacial Maximum, and precedes a major supervolcano eruption in the Mediterranean. Thus, the precise determination of the timing and duration of the Laschamp would help in elucidating major scientific questions situated at the intersection of geology, paleoclimatology, and anthropology. Here we present a geomagnetic record from a stalagmite collected in Crevice Cave, Missouri, which we have dated using a combination of high-precision 230Th ages and annual layer counting using confocal microscopy. We have found a maximum duration for the Laschamp that spans the interval 42,250-39,700 years BP, and an age of 41,100 ± 350 years BP for the height of the excursion. During this period relative paleointensity decreased by an order of magnitude and the virtual geomagnetic pole was located at southerly latitudes. Our chronology provides the first robust bracketing for the Laschamp excursion, and improves on previous age determinations

  15. TRIGGERING COLLAPSE OF THE PRESOLAR DENSE CLOUD CORE AND INJECTING SHORT-LIVED RADIOISOTOPES WITH A SHOCK WAVE. I. VARIED SHOCK SPEEDS

    SciTech Connect

    Boss, Alan P.; Keiser, Sandra A.; Ipatov, Sergei I.; Myhill, Elizabeth A.; Vanhala, Harri A. T. E-mail: keiser@dtm.ciw.ed E-mail: elizabeth.myhill@marymount.ed

    2010-01-10

    The discovery of decay products of a short-lived radioisotope (SLRI) in the Allende meteorite led to the hypothesis that a supernova shock wave transported freshly synthesized SLRI to the presolar dense cloud core, triggered its self-gravitational collapse, and injected the SLRI into the core. Previous multidimensional numerical calculations of the shock-cloud collision process showed that this hypothesis is plausible when the shock wave and dense cloud core are assumed to remain isothermal at approx10 K, but not when compressional heating to approx1000 K is assumed. Our two-dimensional models with the FLASH2.5 adaptive mesh refinement hydrodynamics code have shown that a 20 km s{sup -1} shock front can simultaneously trigger collapse of a 1 M{sub sun} core and inject shock wave material, provided that cooling by molecular species such as H{sub 2}O, CO, and H{sub 2} is included. Here, we present the results for similar calculations with shock speeds ranging from 1 km s{sup -1} to 100 km s{sup -1}. We find that shock speeds in the range from 5 km s{sup -1} to 70 km s{sup -1} are able to trigger the collapse of a 2.2 M{sub sun} cloud while simultaneously injecting shock wave material: lower speed shocks do not achieve injection, while higher speed shocks do not trigger sustained collapse. The calculations continue to support the shock-wave trigger hypothesis for the formation of the solar system, though the injection efficiencies in the present models are lower than desired.

  16. Formation of the Short-lived Radionuclide 36Cl in the Protoplanetary Disk During Late-stage Irradiation of a Volatile-rich Reservoir

    NASA Astrophysics Data System (ADS)

    Jacobsen, Benjamin; Matzel, Jennifer; Hutcheon, Ian D.; Krot, Alexander N.; Yin, Qing-Zhu; Nagashima, Kazuhide; Ramon, Erick C.; Weber, Peter K.; Ishii, Hope A.; Ciesla, Fred J.

    2011-04-01

    Short-lived radionuclides (SLRs) in the early solar system provide fundamental insight into protoplanetary disk evolution. We measured the 36Cl-36S-isotope abundance in wadalite (<15 μm), a secondary chlorine-bearing mineral found in calcium-aluminum-rich inclusions (CAIs) in the Allende CV chondrite, to decipher the origin of the SLR 36Cl (τ 1/2 ~ 3 × 105 yr) in the early solar system. Its presence, initial abundance, and the noticeable decoupling from 26Al raise serious questions about the origin of SLRs. The inferred initial 36Cl abundance for wadalite, corresponding to a 36Cl/35Cl ratio of (1.81 ± 0.13) × 10-5, is the highest 36Cl abundance ever reported in any early solar system material. The high level of 36Cl in wadalite and the absence of 26Al (26Al/27Al <= 3.9 × 10-6) in co-existing grossular (1) unequivocally support the production of 36Cl by late-stage solar energetic particle irradiation in the protoplanetary disk and (2) indicates that the production of 36Cl, recorded by wadalite, is unrelated to the origin of 26Al and other SLRs (10Be, 53Mn) recorded by primary minerals of CAIs and chondrules. We infer that 36Cl was largely produced by irradiation of a volatile-rich reservoir in an optically thin protoplanetary disk adjacent to the region in which the CV chondrite parent asteroid accreted while the Sun was a weak T Tauri star. Subsequently, 36Cl accreted into the Allende CV chondrite together with condensed water ices.

  17. TRIGGERING COLLAPSE OF THE PRESOLAR DENSE CLOUD CORE AND INJECTING SHORT-LIVED RADIOISOTOPES WITH A SHOCK WAVE. II. VARIED SHOCK WAVE AND CLOUD CORE PARAMETERS

    SciTech Connect

    Boss, Alan P.; Keiser, Sandra A. E-mail: keiser@dtm.ciw.edu

    2013-06-10

    A variety of stellar sources have been proposed for the origin of the short-lived radioisotopes that existed at the time of the formation of the earliest solar system solids, including Type II supernovae (SNe), asymptotic giant branch (AGB) and super-AGB stars, and Wolf-Rayet star winds. Our previous adaptive mesh hydrodynamics models with the FLASH2.5 code have shown which combinations of shock wave parameters are able to simultaneously trigger the gravitational collapse of a target dense cloud core and inject significant amounts of shock wave gas and dust, showing that thin SN shocks may be uniquely suited for the task. However, recent meteoritical studies have weakened the case for a direct SN injection to the presolar cloud, motivating us to re-examine a wider range of shock wave and cloud core parameters, including rotation, in order to better estimate the injection efficiencies for a variety of stellar sources. We find that SN shocks remain as the most promising stellar source, though planetary nebulae resulting from AGB star evolution cannot be conclusively ruled out. Wolf-Rayet (WR) star winds, however, are likely to lead to cloud core shredding, rather than to collapse. Injection efficiencies can be increased when the cloud is rotating about an axis aligned with the direction of the shock wave, by as much as a factor of {approx}10. The amount of gas and dust accreted from the post-shock wind can exceed that injected from the shock wave, with implications for the isotopic abundances expected for a SN source.

  18. 2014 ICHLNRRA intercomparison of radon/thoron gas and radon short-lived decay products measuring instruments in the NRPI Prague.

    PubMed

    Jílek, K; Timková, J

    2015-06-01

    During the Eighth International Conference on High Levels of Natural Radiation and Radon Areas held in autumn 2014 at Prague, the third intercomparison of radon/thoron gas and radon short-lived decay products measurement instruments was organised by and held at the Natural Radiation Division of the National Radiation Protection Institute (NRPI; SÚRO v.v.i.) in Prague. The intercomparison was newly focussed also on continuous monitors with active sampling adapters capable to distinguish radon/thoron gas in their mix field.The results of radon gas measurements carried out in the big NRPI radon chamber indicated very well an average deviation of up to 5 % from the reference NRPI value for 80 % of all the exposed instruments. The results of equilibrium equivalent concentration continuous monitors indicated an average deviation of up to 5 % from the reference NRPI value for 40 % of all the exposed instruments and their ~8-10 % shift compared with the NRPI. The results of investigated ambient conditions upon response of exposed continuous monitors indicated influence of aerosol changes upon response of radon monitors with an active air sampling adapters through the filter, only. The exposures of both radon/thoron gas discriminative continuous monitors and passive detectors have been indicated inconsistent results: on one hand, their excellent agreement up to several per cent for both the gases, and on the other hand, systematic unsatisfactory differences up to 40 %. Additional radon/thoron exercises are recommended to improve both the instruments themselves and quality of their operators. PMID:25990114

  19. Brick Kiln Emissions Quantified with the Aerodyne Mobile Laboratory During the Short Lived Climate Forcing (SLCF) 2013 Campaign in Guanajuato Mexico

    NASA Astrophysics Data System (ADS)

    Fortner, E.; Knighton, W. B.; Herndon, S.; Roscioli, J. R.; Zavala, M.; Onasch, T. B.; Jayne, J. T.; Worsnop, D. R.; Kolb, C. E.; Molina, L. T.

    2013-12-01

    Brick kiln emissions are suspected to be a major source of atmospheric black carbon (BC) in developing countries; and black carbon's role as a short lived climate forcing (SLCF) pollutant is widely recognized. The SLCF-Mexico brick kiln study was conducted from 12-17 March 2013 in Mexico's Guanajuato state. Three different types of brick kilns were investigated (MK2, traditional, and traditional three tier) providing data on the effects of different kiln designs on particle and gas phase emissions. The BC and gaseous combustion emissions from these kilns were measured during both the fire stage and the subsequent smoldering stage with real-time instruments deployed on the Aerodyne Mobile Laboratory, and quantified utilizing flux tracer gases released adjacent to the brick kiln. This method allows examination of the brick kiln plume's evolution as it transits downwind from the source. Particulate measurements conducted by the mobile laboratory included the multi angle absorption photometer (MAAP) to measure black carbon mass, cavity attenuated phase shift (CAPSext) monitor to measure extinction and soot particle aerosol mass spectrometer (SP-AMS) measurements of black carbon. The SP-AMS instrument combines the ability to measure black carbon with the ability to determine the chemical composition of the other particulate matter (PM) components associated with black carbon particles. The variance of PM chemical composition will be examined as a function of burning stage and kiln type and compared to other black carbon PM sources. Gas phase exhaust species measured included CO, CO2, NOx, SO2, CH4, C2H6, as well as a variety of VOCs (acetonitrile, benzene etc.) measured with a PTR-MS instrument. All of these measurements will be examined to construct emission ratios evaluating how these vary with different kiln types and different firing conditions. The evolution of particulate matter and gas phase species as they transit away from the source will also be examined.

  20. A Lower Initial Abundance of Short-lived 41Ca in the Early Solar System and Its Implications for Solar System Formation

    NASA Astrophysics Data System (ADS)

    Liu, Ming-Chang; Chaussidon, Marc; Srinivasan, Gopalan; McKeegan, Kevin D.

    2012-12-01

    The short-lived radionuclide 41Ca plays an important role in constraining the immediate astrophysical environment and the formation timescale of the nascent solar system due to its extremely short half-life (0.1 Myr). Nearly 20 years ago, the initial ratio of 41Ca/40Ca in the solar system was determined to be (1.41 ± 0.14) × 10-8, primarily based on two Ca-Al-rich Inclusions (CAIs) from the CV chondrite Efremovka. With an advanced analytical technique for isotopic measurements, we reanalyzed the potassium isotopic compositions of the two Efremovka CAIs and inferred the initial ratios of 41Ca/40Ca to be (2.6 ± 0.9) × 10-9 and (1.4 ± 0.6) × 10-9 (2σ), a factor of 7-10 lower than the previously inferred value. Considering possible thermal processing that led to lower 26Al/27Al ratios in the two CAIs, we propose that the true solar system initial value of 41Ca/40Ca should have been ~4.2 × 10-9. Synchronicity could have existed between 26Al and 41Ca, indicating a uniform distribution of the two radionuclides at the time of CAI formation. The new initial 41Ca abundance is 4-16 times lower than the calculated value for steady-state galactic nucleosynthesis. Therefore, 41Ca could have originated as part of molecular cloud materials with a free decay time of 0.2-0.4 Myr. Alternative possibilities, such as a last-minute input from a stellar source and early solar system irradiation, could not be definitively ruled out. This underscores the need for more data from diverse CAIs to determine the true astrophysical origin of 41Ca.

  1. Stepwise Catalytic Mechanism via Short-Lived Intermediate Inferred from Combined QM/MM MERP and PES Calculations on Retaining Glycosyltransferase ppGalNAcT2

    PubMed Central

    Trnka, Tomáš; Kozmon, Stanislav; Tvaroška, Igor; Koča, Jaroslav

    2015-01-01

    The glycosylation of cell surface proteins plays a crucial role in a multitude of biological processes, such as cell adhesion and recognition. To understand the process of protein glycosylation, the reaction mechanisms of the participating enzymes need to be known. However, the reaction mechanism of retaining glycosyltransferases has not yet been sufficiently explained. Here we investigated the catalytic mechanism of human isoform 2 of the retaining glycosyltransferase polypeptide UDP-GalNAc transferase by coupling two different QM/MM-based approaches, namely a potential energy surface scan in two distance difference dimensions and a minimum energy reaction path optimisation using the Nudged Elastic Band method. Potential energy scan studies often suffer from inadequate sampling of reactive processes due to a predefined scan coordinate system. At the same time, path optimisation methods enable the sampling of a virtually unlimited number of dimensions, but their results cannot be unambiguously interpreted without knowledge of the potential energy surface. By combining these methods, we have been able to eliminate the most significant sources of potential errors inherent to each of these approaches. The structural model is based on the crystal structure of human isoform 2. In the QM/MM method, the QM region consists of 275 atoms, the remaining 5776 atoms were in the MM region. We found that ppGalNAcT2 catalyzes a same-face nucleophilic substitution with internal return (SNi). The optimized transition state for the reaction is 13.8 kcal/mol higher in energy than the reactant while the energy of the product complex is 6.7 kcal/mol lower. During the process of nucleophilic attack, a proton is synchronously transferred to the leaving phosphate. The presence of a short-lived metastable oxocarbenium intermediate is likely, as indicated by the reaction energy profiles obtained using high-level density functionals. PMID:25849117

  2. RNA-seq of the aging brain in the short-lived fish N. furzeri – conserved pathways and novel genes associated with neurogenesis

    PubMed Central

    Baumgart, Mario; Groth, Marco; Priebe, Steffen; Savino, Aurora; Testa, Giovanna; Dix, Andreas; Ripa, Roberto; Spallotta, Francesco; Gaetano, Carlo; Ori, Michela; Terzibasi Tozzini, Eva; Guthke, Reinhard; Platzer, Matthias; Cellerino, Alessandro

    2014-01-01

    The brains of teleost fish show extensive adult neurogenesis and neuronal regeneration. The patterns of gene regulation during fish brain aging are unknown. The short-lived teleost fish Nothobranchius furzeri shows markers of brain aging including reduced learning performances, gliosis, and reduced adult neurogenesis. We used RNA-seq to quantify genome-wide transcript regulation and sampled five different time points to characterize whole-genome transcript regulation during brain aging of N. furzeri. Comparison with human datasets revealed conserved up-regulation of ribosome, lysosome, and complement activation and conserved down-regulation of synapse, mitochondrion, proteasome, and spliceosome. Down-regulated genes differ in their temporal profiles: neurogenesis and extracellular matrix genes showed rapid decay, synaptic and axonal genes a progressive decay. A substantial proportion of differentially expressed genes (∼40%) showed inversion of their temporal profiles in the last time point: spliceosome and proteasome showed initial down-regulation and stress-response genes initial up-regulation. Extensive regulation was detected for chromatin remodelers of the DNMT and CBX families as well as members of the polycomb complex and was mirrored by an up-regulation of the H3K27me3 epigenetic mark. Network analysis showed extensive coregulation of cell cycle/DNA synthesis genes with the uncharacterized zinc-finger protein ZNF367 as central hub. In situ hybridization showed that ZNF367 is expressed in neuronal stem cell niches of both embryonic zebrafish and adult N. furzeri. Other genes down-regulated with age, not previously associated with adult neurogenesis and with similar patterns of expression are AGR2, DNMT3A, KRCP, MEX3A, SCML4, and CBX1. CBX7, on the other hand, was up-regulated with age. PMID:25059688

  3. Preliminary Results of IS Plasma Focus as a Breeder of Short-Lived Radioisotopes 12C(d,n)13N

    NASA Astrophysics Data System (ADS)

    Sadat Kiai, S. M.; Elahi, M.; Adlparvar, S.; Shahhoseini, E.; Sheibani, S.; Ranjber akivaj, H.; Alhooie, S.; Safarien, A.; Farhangi, S.; Aghaei, N.; Amini, S.; Khalaj, M. M.; Zirak, A. R.; Dabirzadeh, A. A.; Soleimani, J.; Torkzadeh, F.; Mousazadeh, M. M.; Moradi, K.; Abdollahzadeh, M.; Talaei, A.; Zaeem, A. A.; Moslehi, A.; Kashani, A.; Babazadeh, A. R.; Bagiyan, F.; Ardestani, M.; Roozbahani, A.; Pourbeigi, H.; Tajik Ahmadi, H.; Ahmadifaghih, M. A.; Mahlooji, M. S.; Mortazavi, B. N.; Zahedi, F.

    2011-04-01

    Modified IS (Iranian Sun) plasma focus (10 kJ,15 kV, 94 μF, 0.1 Hz) has been used to produce the short-lived radioisotope 13N (half-life of 9.97 min) through 12C(d,n)13N nuclear reaction. The filling gas was 1.5-3 torr of hydrogen (60%) deuterium (40%) mixture. The target was solid nuclear grade graphite with 5 mm thick, 9 cm width and 13 in length. The activations of the exogenous target on average of 20 shots (only one-third acceptable) through 10-13 kV produced the 511 keV gamma rays. Another peak found at the 570 keV gamma of which both was measured by a NaI portable gamma spectrometer calibrated by a 137Cs 0.25 μCi sealed reference source with its single line at 661.65 keV and 22Na 0.1 μCi at 511 keV. To measure the gamma rays, the graphite target converts to three different phases; solid graphite, powder graphite, and powder graphite in water solution. The later phase approximately has a doubled activity with respect to the solid graphite target up to 0.5 μCi of 511 keV and 1.1 μCi of 570 keV gamma lines were produced. This increment in activity was perhaps due to structural transformation of graphite powder to nano-particles characteristic in liquid water.

  4. FORMATION OF THE SHORT-LIVED RADIONUCLIDE {sup 36}Cl IN THE PROTOPLANETARY DISK DURING LATE-STAGE IRRADIATION OF A VOLATILE-RICH RESERVOIR

    SciTech Connect

    Jacobsen, Benjamin; Yin Qingzhu; Matzel, Jennifer; Hutcheon, Ian D.; Ramon, Erick C.; Weber, Peter K.; Krot, Alexander N.; Nagashima, Kazuhide; Ishii, Hope A.; Ciesla, Fred J.

    2011-04-20

    Short-lived radionuclides (SLRs) in the early solar system provide fundamental insight into protoplanetary disk evolution. We measured the {sup 36}Cl-{sup 36}S-isotope abundance in wadalite (<15 {mu}m), a secondary chlorine-bearing mineral found in calcium-aluminum-rich inclusions (CAIs) in the Allende CV chondrite, to decipher the origin of the SLR {sup 36}Cl ({tau}{sub 1/2} {approx} 3 x 10{sup 5} yr) in the early solar system. Its presence, initial abundance, and the noticeable decoupling from {sup 26}Al raise serious questions about the origin of SLRs. The inferred initial {sup 36}Cl abundance for wadalite, corresponding to a {sup 36}Cl/{sup 35}Cl ratio of (1.81 {+-} 0.13) x 10{sup -5}, is the highest {sup 36}Cl abundance ever reported in any early solar system material. The high level of {sup 36}Cl in wadalite and the absence of {sup 26}Al ({sup 26}Al/{sup 27}Al {<=} 3.9 x 10{sup -6}) in co-existing grossular (1) unequivocally support the production of {sup 36}Cl by late-stage solar energetic particle irradiation in the protoplanetary disk and (2) indicates that the production of {sup 36}Cl, recorded by wadalite, is unrelated to the origin of {sup 26}Al and other SLRs ({sup 10}Be, {sup 53}Mn) recorded by primary minerals of CAIs and chondrules. We infer that {sup 36}Cl was largely produced by irradiation of a volatile-rich reservoir in an optically thin protoplanetary disk adjacent to the region in which the CV chondrite parent asteroid accreted while the Sun was a weak T Tauri star. Subsequently, {sup 36}Cl accreted into the Allende CV chondrite together with condensed water ices.

  5. The Multi-Temporal Database of Planetary Image Data (MUTED): A database to support the identification of surface changes and short-lived surface processes

    NASA Astrophysics Data System (ADS)

    Erkeling, G.; Luesebrink, D.; Hiesinger, H.; Reiss, D.; Heyer, T.; Jaumann, R.

    2016-06-01

    Images of Mars taken by spacecraft in the last few decades indicate that the landscape has changed and that current processes are continuously changing the surface. The modifications of the landscape are caused by exogenic processes including eolian activity, mass movement, the growth and retreat of the polar caps, glacial processes and crater-forming impacts. In particular the High Resolution Stereo Camera (HRSC) on board Mars Express (MEx) and the Context Camera (CTX) on board the Mars Reconnaissance Orbiter (MRO) cover large areas at high resolution and thus are particularly well-suited to detect the extent and origin of surface changes on Mars. Multi-temporal observations of variable features on Mars became possible by the increasing number of repeated image acquisitions of the same surface areas. To support the investigation of surface changes that represents a key element in martian research, we developed MUTED, the "Multi-Temporal Database of Planetary Image Data", which is a tool for the identification of the spatial and multi-temporal coverage of planetary image data from Mars. Using MUTED, scientists are able to identify the location, number, and time range of acquisitions of overlapping images from, for example, HRSC and CTX. MUTED also includes images from other planetary datasets such as those of the Mars Orbiter Camera (MOC), the Thermal Emission Imaging System (THEMIS), and the High Resolution Imaging Science Experiment (HiRISE). The database supports the identification and analysis of surface changes and short-lived surface processes on Mars based on fast automatic planetary image database queries. From the multi-temporal planetary image database and investigations based on multi-temporal observations we will better understand the interactions between the surface of Mars and external forces, including the atmosphere. MUTED is available for the planetary scientific community via the webpage of the Institut für Planetologie (IfP) Muenster.

  6. Neutron Capture Cross Sections for Radioactive Nuclei

    NASA Astrophysics Data System (ADS)

    Tonchev, Anton; Bedrossian, Peter; Escher, Jutta; Scielzo, Nicholas

    2015-10-01

    Accurate neutron-capture cross sections for radioactive nuclei near or far away from the line of beta stability are crucial for understanding the nucleosynthesis of heavy elements. However, neutron-capture cross sections for short-lived radionuclides are difficult to measure due to the fact that the measurements require both highly radioactive samples and intense neutron sources. Essential ingredients for describing the γ decays following neutron capture are the γ-ray strength function and level densities. We will compare different indirect approaches for obtaining observables that can constrain Hauser-Feshbach statistical model calculations of capture cross sections. Specifically, we will consider photon scattering, transfer reactions, and beta-delayed neutron emission. Challenges that exist on the path to obtaining neutron-capture cross sections for reactions on isotopes far from stability will be discussed. This work was performed under the auspices of US DOE by LLNL under contract DE-AC52-07NA27344. Funding was provided via the LDRD-ERD-069 project.

  7. Experiments with Superheavy Nuclei

    NASA Astrophysics Data System (ADS)

    Hofmann, S.

    1999-03-01

    In two series of experiments at SHIP, six new elements (Z=107-112) were synthesized via fusion reactions using lead or bismuth targets and 1n-deexcitation channels. The isotopes were unambiguously identified by means of α -α correlations. Not fission, but alpha decay is the dominant decay mode. Cross-sections decrease by two orders of magnitude from bohrium (Z=107) to element 112, for which a cross-section of 1 pb was measured. Based on these results, it is likely that the production of isotopes of element 114 close to the island of spherical SuperHeavy Elements (SHE) could be achieved by fusion reactions using 208Pb targets. Systematic studies of the reaction cross-sections indicate that the transfer of nucleons is an important process for the initiation of fusion. The data allow for the fixing of a narrow energy window for the production of SHE using 1n-emission channels. The likelihood of broadening the energy window by investigation of radiative capture reactions, use of neutron deficient projectile isotopes and use of actinide targets is discussed.

  8. Formation of short-lived radionuclides in the protoplanetary disk during late-stage irradiation of a volatile-rich reservoir

    SciTech Connect

    Jacobsen, B; Matzel, J; Hutcheon, I D; Krot, A N; Yin, Q -; Nagashima, K; Ramon, E; Weber, P; Ishii, H; Ciesla, F

    2010-11-30

    The origin of short-lived (t{sub 1/2} < 5 Myr) and now extinct radionuclides ({sup 10}Be, {sup 26}Al, {sup 36}Cl, {sup 41}Ca, {sup 53}Mn, {sup 60}Fe; hereafter SLRs) is fundamental to understanding the formation of the early solar system. Two distinct classes of models have been proposed to explain the origin of SLRs: (1) injection from a nearby stellar source (e.g., supernova, asymptotic giant branch star or Wolf-Rayet star) and (2) solar energetic particle irradiation of dust and gas near the proto-Sun. Recent studies have demonstrated that {sup 36}Cl was extant in the early solar system. However, its presence, initial abundance and the noticeable decoupling from {sup 26}Al raise serious questions about the origin of SLRs. Here we report {sup 36}Cl-{sup 36}S and {sup 26}Al-{sup 26}Mg systematics for wadalite and grossular, secondary minerals in a calcium-aluminum-rich inclusion (CAI) from the CV chondrite Allende that allow us to reassess the origin of SLRs. The inferred abundance of {sup 36}Cl in wadalite, corresponding to a {sup 36}Cl/{sup 35}Cl ratio of (1.81 {+-} 0.13) x 10{sup -5}, is the highest {sup 36}Cl abundance reported in any early solar system material. The high level of {sup 36}Cl in wadalite and the absence of {sup 26}Al ({sup 26}Al/{sup 27}Al {le} 3.9 x 10{sup -6}) in co-existing grossular indicates that (1) {sup 36}Cl formed by late-stage solar energetic particle irradiation and (2) the production of {sup 36}Cl, recorded by secondary minerals, is unrelated to the origin of {sup 26}Al and other SLRs ({sup 10}Be, {sup 53}Mn) recorded by primary minerals of CAIs and chondrules. We conclude that 36Cl was produced by solar energetic particle irradiation of a volatile-rich reservoir in an optically thin protoplanetary disk adjacent to the accretion region of the CV chondrite parent asteroid.

  9. Determination of the cross section for (n,p) reaction with producing short-lived nuclei on the 162,163Dy isotopes at 13.5 and 14.8 MeV

    NASA Astrophysics Data System (ADS)

    Luo, Junhua; Feng, Zhifu; An, Li; Jiang, Li; He, Long

    2016-06-01

    Activation cross-sections for the 162Dy(n,p)162Tb and 163Dy(n,p)163Tb reactions have been measured by means of the activation technique and a coaxial HPGe γ-ray detector at 13.5 and 14.8 MeV. The fast neutrons were produced via the 3H(d,n)4He reaction on Pd-300 neutron generator. The natural high-purity Dy2O3 powder was used as target material. Theoretical excitation functions were calculated using the nuclear-reaction codes EMPIRE-3.2 Malta and TALYS-1.6 with default parameters, at neutron energies varying from the reaction threshold to 20 MeV. The results were also discussed and compared with some corresponding values found in the literature, with the comprehensive evaluation data in ENDF/B-VII.1 and JENDF-4.0 libraries, and with the estimates obtained from a published empirical formula based on the statistical model with Q-value dependence and odd-even effects taken into consideration.

  10. Heavy nuclei far from stability in the N < 126, Z > 82 region

    SciTech Connect

    Back, B.B.; Blumenthal, D.J.; Carpenter, M.P.

    1995-08-01

    There are long-standing calculations suggesting that nuclei in the N < 126, Z > 82 region far from stability exhibit deformation effects. Away from stability an observable permanent quadrupole deformation should be achieved but, as yet, there is no experimental evidence for such an effect. A series of experiments was performed to assess the production of nuclei in this region and to study their structure. These experiments were performed using gamma-ray spectroscopy to investigate the low-lying level schemes and alpha-particle spectroscopy in order to isolate fine structure in the decay. The low-lying level structure of the neutron-deficient isotope {sup 202}Rn was studied, for the first time, using the {sup 181}Ta({sup 27}Al,6n) and {sup 192}Pt({sup 16}O,6n) reactions. Gamma-ray transitions between excited states in {sup 202}Rn were identified by mass tagging the Fragment Mass Analyzer and by observation of coincident X rays. Transitions in {sup 203}Rn were also identified. The level scheme deduced from these data is consistent with the systematics of light radon isotopes below the N = 126 shell closure and with theoretical calculations indicating that the ground-state shape should not be strongly deformed at N = 116.

  11. Assessing and modeling sediment mobility in estuarine and coastal settings due to extreme climate events from natural short-lived isotope distribution

    NASA Astrophysics Data System (ADS)

    Ghaleb, Bassam; Hillaire-Marcel, Claude; Ruiz Fernandez, Ana-Carolina; Sanchez Cabeza, Joan-Albert

    2016-04-01

    Climatic events (e.g. floods, storminess) and management activities (e.g. dredging) may result in the burial or removal and re-suspension of sediments in estuaries and coastal areas. When such sediments are contaminated, such processes may either help restoring better chemical environments or lead to their long-term contamination. Geochemical signatures in surface sediments may help identifying such sedimentological events. However, short-lived isotope data are generally required to set time-constraints on their occurrence. Whereas 210Pb and radioactive fallout isotope contents can help setting time constraints at ~50 to ~100 yr-time scales, natural disequilibria in the 232Th-228Ra-228Th sequence do provide information on processes which occurred within the last 30 yrs, as illustrated in the present study. Box-cored sediments from the Saguenay Fjord and lower estuary of the St. Lawrence (Canada) as well as from estuaries and lagoons from the Sinaloa Coast (Mexico) are used to document the behavior of these isotopes either under relatively steady conditions (St. Lawrence estuary) or under high-frequency extreme climate events (storms and floods; Saguenay Fjord, Coastal Sinaloa). 228Th/232Th activity ratios were determined by chemical extraction of Th and alpha counting of unspiked samples, rapidly after sampling (228Th/232Th). The activity of the intermediate isotope 228Ra was then estimated based on replicate measurements on aliquot samples made a few years later. Under steady conditions, core-top sediment shows an excess in 228Th vs 232Th (AR ~ 1.6), whereas the intermediate 228Ra depicts a deficit vs its parent 232Th (AR ~0.6). Downcore, radioactive decay carries rapidly 228Th-activities to those of the parent 228Ra within about 10 yrs (i.e., ~ 5 half-lives of 228Th), then both move during the next ~20 yrs (~ i.e., ~ 5 half-lives of 228Ra, when added to the 10 yrs of 228Th-excess) towards secular equilibrium with the parent long-lived 232Th. A few algorithms

  12. Oxygen isotopic and geochemical evidence for a short-lived, high-temperature hydrothermal event in the Chegem caldera, Caucasus Mountains, Russia

    USGS Publications Warehouse

    Gazis, C.; Taylor, H.P., Jr.; Hon, K.; Tsvetkov, A.

    1996-01-01

    Within the 2.8 Ma Chegem ash-flow caldera (11 ?? 15 km), a single cooling unit of rhyolitic to dacitic welded tuff more than 2 km thick is exposed in deep valleys incised during recent rapid uplift of the Caucasus Mountains. The intracaldera tuff is mineralogically fresh and unaltered, and is overlain by andesite lavas and cut by a resurgent granodiorite intrusion. Major- and trace-element compositions for a 1405-m stratigraphic section of intracaldera tuff display trends of upwardly increasing Na2O, CaO, Al2O3, total Fe, MgO, TiO2, Sr and Zr and decreasing SiO2, K2O and Rb. This mafic-upward zoning (from 76.1 to 69.9% SiO2) reflects an inverted view of the upper part of the source magma chamber. Oxygen isotope studies of 35 samples from this 1405-m section define a striking profile with "normal" igneous ??18O values (+7.0 to +8.5) in the lower 600 m of tuff, much lower ??18O values (-4.0 to +4.3) in a 700-m zone above that and a shift to high ??18O values (+4.4 to -10.9) in the upper 100 m of caldera-fill exposure. Data from two other partial stratigraphic sections indicate that these oxygen isotope systematics are probably a caldera-wide phenomenon. Quartz and feldspar phenocrysts everywhere have "normal" igneous ??18O values of about +8.5 and +7.5, respectively, whereas groundmass and glass ??18O values range from -7.7 to +12.3. Consequently, the ??18O values of coexisting feldspar, groundmass and glass form a steep array in a plot of ??feldspar vs. ??groundmass/glass. Such pronounced disequilibrium between coexisting feldspar and groundmass or glass has never before been observed on this scale. It requires a hydrothermal event involving large amounts of low-18O H2O at sufficiently high temperatures and short enough time (tens of years or less) that glass exchanges thoroughly but feldspar does not. The most likely process responsible for the O depletions at Chegem is a very high temperature (500-600??C), short-lived, vigorous meteoric-hydrothermal event that was

  13. Active galactic nuclei

    PubMed Central

    Fabian, Andrew C.

    1999-01-01

    Active galactic nuclei are the most powerful, long-lived objects in the Universe. Recent data confirm the theoretical idea that the power source is accretion into a massive black hole. The common occurrence of obscuration and outflows probably means that the contribution of active galactic nuclei to the power density of the Universe has been generally underestimated. PMID:10220363

  14. Structure Of Rare-Earth Nuclei Around The Proton Drip Line

    SciTech Connect

    Rykaczewski, K.P.; Gross, C.J.; Yu, C.H.; Grzywacz, R.K.; Bingham, C.R.; Danchev, M.; Mazzocchi, C.; Tantawy, M.N.; Batchelder, J.C.; Karny, M.; Krolas, W.; Fong, D.; Hamilton, J.H.; Ramayya, A.V.; Piechaczek, A.; Zganjar, E.; Winger, J.A.; Ginter, T.N.; Stolz, A.; Hagino, K.

    2005-04-05

    Decay studies on rare earth nuclei around the proton drip line have been performed by means of the Recoil Mass Spectrometer at the Holifield Radioactive Ion Beam Facility in Oak Ridge. The proton emission from the odd-odd N=77 isotone 146Tm was reinvestigated, resulting in the assignment of the 1.01 MeV proton line to the decay of a short-lived 146Tm state. A new proton radioactivity of 144Tm was identified. The decays of isomeric levels in the N=77 isotones, 140Eu, 142Tb and 144Ho were remeasured using {gamma} and electron detectors. The analysis of the structure of studied nuclei, which accounts for the coupling between the protons and neutrons and for core excitations, is presented.

  15. Distributions of Long-lived Radioactive Nuclei Provided by Star-forming Environments

    NASA Astrophysics Data System (ADS)

    Fatuzzo, Marco; Adams, Fred C.

    2015-11-01

    Radioactive nuclei play an important role in planetary evolution by providing an internal heat source, which affects planetary structure and helps facilitate plate tectonics. A minimum level of nuclear activity is thought to be necessary—but not sufficient—for planets to be habitable. Extending previous work that focused on short-lived nuclei, this paper considers the delivery of long-lived radioactive nuclei to circumstellar disks in star forming regions. Although the long-lived nuclear species are always present, their abundances can be enhanced through multiple mechanisms. Most stars form in embedded cluster environments, so that disks can be enriched directly by intercepting ejecta from supernovae within the birth clusters. In addition, molecular clouds often provide multiple episodes of star formation, so that nuclear abundances can accumulate within the cloud; subsequent generations of stars can thus receive elevated levels of radioactive nuclei through this distributed enrichment scenario. This paper calculates the distribution of additional enrichment for 40K, the most abundant of the long-lived radioactive nuclei. We find that distributed enrichment is more effective than direct enrichment. For the latter mechanism, ideal conditions lead to about 1 in 200 solar systems being directly enriched in 40K at the level inferred for the early solar nebula (thereby doubling the abundance). For distributed enrichment from adjacent clusters, about 1 in 80 solar systems are enriched at the same level. Distributed enrichment over the entire molecular cloud is more uncertain, but can be even more effective.

  16. Exotic Light Nuclei

    ERIC Educational Resources Information Center

    Cerny, Joseph; Poskanzer, Arthur M.

    1978-01-01

    Among the light elements, nuclei with unequal numbers of protons and neutrons are highly unstable. Some survive just long enough to be detected and exhibit unusual regimes of radioactive decay. ( Autor/MA)

  17. Isotope shifts of the 6d{sup 2} D{sub 3/2}-7 p{sup 2} P{sub 1/2} transition in trapped short-lived {sup 209-214}Ra{sup +}

    SciTech Connect

    Giri, G. S.; Versolato, O. O.; Berg, J. E. van den; Boell, O.; Dammalapati, U.; Hoek, D. J. van der; Jungmann, K.; Kruithof, W. L.; Mueller, S.; Nunez Portela, M.; Onderwater, C. J. G.; Santra, B.; Timmermans, R. G. E.; Wansbeek, L. W.; Willmann, L.; Wilschut, H. W.

    2011-08-15

    Laser spectroscopy of short-lived radium isotopes in a linear Paul trap has been performed. The isotope shifts of the 6d{sup 2} D{sub 3/2} -7 p{sup 2} P{sub 1/2} transition in {sup 209-214}Ra{sup +}, which are sensitive to the short-range part of the atomic wave functions, were measured. The results are essential experimental input for improving the precision of atomic structure calculations. This is indispensable for parity violation in Ra{sup +} aiming at the determination of the weak mixing angle.

  18. Production of heavy and superheavy neutron-rich nuclei in transfer reactions

    SciTech Connect

    Zagrebaev, V. I.; Greiner, Walter

    2011-04-15

    The problem of production and study of heavy neutron-rich nuclei has been intensively discussed during recent years. Many reasons arouse a great interest in this problem. The present limits of the upper part of the nuclear map are very close to the {beta} stability line while the unexplored area of heavy neutron-rich nuclides (also those located along the neutron closed shell N=126 to the right-hand side of the stability line) is extremely important for nuclear astrophysic investigations and, in particular, for the understanding of the r process of astrophysical nucleogenesis. For elements with Z>100 only neutron deficient isotopes (located to the left of the stability line) have been synthesized so far. The 'northeast' area of the nuclear map can be reached neither in fusion-fission reactions nor in fragmentation processes widely used nowadays for the production of new nuclei. Multinucleon transfer processes in near barrier collisions of heavy (and very heavy, U-like) ions seem to be the only reaction mechanism allowing us to produce and explore neutron-rich heavy nuclei including those located at the superheavy island of stability. In this paper several transfer reactions for different projectile-target combinations are studied in detail. Besides the predictions for the cross sections of such processes, we also analyze the angular and energy distributions of primary and survived reaction products in the laboratory frame. These results, as well as predicted excitation functions for the yields of neutron-rich superheavy isotopes, might be useful for the design of appropriate experimental equipment and for carrying out experiments of such kind.

  19. Radiations from hot nuclei

    NASA Technical Reports Server (NTRS)

    Malik, F. Bary

    1993-01-01

    The investigation indicates that nuclei with excitation energy of a few hundred MeV to BeV are more likely to radiate hot nuclear clusters than neutrons. These daughter clusters could, furthermore, de-excite emitting other hot nuclei, and the chain continues until these nuclei cool off sufficiently to evaporate primarily neutrons. A few GeV excited nuclei could radiate elementary particles preferentially over neutrons. Impact of space radiation with materials (for example, spacecraft) produces highly excited nuclei which cool down emitting electromagnetic and particle radiations. At a few MeV excitation energy, neutron emission becomes more dominant than gamma-ray emission and one often attributes the cooling to take place by successive neutron decay. However, a recent experiment studying the cooling process of 396 MeV excited Hg-190 casts some doubt on this thinking, and the purpose of this investigation is to explore the possibility of other types of nuclear emission which might out-compete with neutron evaporation.

  20. Physics of Unstable Nuclei

    NASA Astrophysics Data System (ADS)

    Khoa, Dao Tien; Egelhof, Peter; Gales, Sydney; Giai, Nguyen Van; Motobayashi, Tohru

    2008-04-01

    Studies at the RIKEN RI beam factory / T. Motobayashi -- Dilute nuclear states / M. Freer -- Studies of exotic systems using transfer reactions at GANIL / D. Beaumel et al. -- First results from the Magnex large-acceptance spectrometer / A. Cunsolo et al. -- The ICHOR project and spin-isospin physics with unstable beams / H. Sakai -- Structure and low-lying states of the [symbol]He exotic nucleus via direct reactions on proton / V. Lapoux et al. -- Shell gap below [symbol]Sn based on the excited states in [symbol]Cd and [symbol]In / M. Górska -- Heavy neutron-rich nuclei produced in the fragmentation of a [symbol]Pb beam / Zs. Podolyák et al. -- Breakup and incomplete fusion in reactions of weakly-bound nuclei / D.J. Hinde et al. -- Excited states of [symbol]B and [symbol]He and their cluster aspect / Y. Kanada-En'yo et al. -- Nuclear reactions with weakly-bound systems: the treatment of the continuum / C. H. Dasso, A. Vitturi -- Dynamic evolution of three-body decaying resonances / A. S. Jensen et al. -- Prerainbow oscillations in [symbol]He scattering from the Hoyle state of [symbol]C and alpha particle condensation / S. Ohkubo, Y. Hirabayashi -- Angular dispersion behavior in heavy ion elastic scattering / Q. Wang et al. -- Microscopic optical potential in relativistic approach / Z.Yu. Ma et al. -- Exotic nuclei studied in direct reactions at low momentum transfer - recent results and future perspectives at fair / P. Egelhof -- Isotopic temperatures and symmetry energy in spectator fragmentation / M. De Napoli et al. -- Multi-channel algebraic scattering theory and the structure of exotic compound nuclei / K. Amos et al. -- Results for the first feasibility study for the EXL project at the experimental storage ring at GSI / N. Kalantar-Nayestanaki et al. -- Coulomb excitation of ISOLDE neutron-rich beams along the Z = 28 chain / P. Van Duppen -- The gamma decay of the pygmy resonance far from stability and the GDR at finite temperature / G. Benzoni et al

  1. Scattering Of Light Nuclei

    SciTech Connect

    Quaglioni, S; Navratil, P; Roth, R

    2009-12-15

    The exact treatment of nuclei starting from the constituent nucleons and the fundamental interactions among them has been a long-standing goal in nuclear physics. Above all nuclear scattering and reactions, which require the solution of the many-body quantum-mechanical problem in the continuum, represent an extraordinary theoretical as well as computational challenge for ab initio approaches.We present a new ab initio many-body approach which derives from the combination of the ab initio no-core shell model with the resonating-group method [4]. By complementing a microscopic cluster technique with the use of realistic interactions, and a microscopic and consistent description of the nucleon clusters, this approach is capable of describing simultaneously both bound and scattering states in light nuclei. We will discuss applications to neutron and proton scattering on sand light p-shell nuclei using realistic nucleon-nucleon potentials, and outline the progress toward the treatment of more complex reactions.

  2. Response of hot nuclei

    SciTech Connect

    Broglia, R.A.

    1986-01-01

    The dipole giant resonance is reviewed, as it is the only vibration which has been experimentally identified in the decay of hot nuclei. The mechanism of exciting the resonance and the mode of the resonance are described. The methods used to calculate the vibrations from the shell model are discussed, including the Hartree-Fock approximation and random phase approximation. Nuclei formed by compound nuclear reactions, which possess high excitation energy and angular momentum, are considered. It is argued that the stability of the dipole may be used to advantage in the study of other properties of nuclei at high excitation. It is also considered possible that the discussion of the dipole giant resonance may be extended to the gamma decay of the isovector quadrupole vibration. 26 refs., 18 figs. (LEW)

  3. Super-heavy nuclei

    NASA Astrophysics Data System (ADS)

    Hofmann, Sigurd

    2015-11-01

    Scientifically based searches for elements beyond uranium started after the discovery of the neutron. Neutrons captured by uranium nuclei and subsequent {β }- decay, similarly as most of the elements were produced in nature, was the successful method applied. However, as a first result, Hahn and Strassmann discovered nuclear fission indicating a limit for the existence of nuclei at an increasing number of protons. Eventually, the nuclear shell model allowed for a more accurate calculation of binding energies, half-lives and decay modes of the heaviest nuclei. Theoreticians predicted a region of increased stability at proton number Z = 126, later shifted to 114, and neutron number N = 184. These nuclei receive their stability from closed shells for the protons and neutrons. Later, increased stability was also predicted for deformed nuclei at Z = 108 and N = 162. In this review I will report on experimental work performed on research to produce and identify these super-heavy nuclei (SHN). Intensive heavy ion beams, sophisticated target technology, efficient electromagnetic ion separators, and sensitive detector arrays were the prerequisites for discovery of 12 new elements during the last 40 years. The results are described and compared with theoretical predictions and interpretations. An outlook is given on further improvement of experimental facilities which will be needed for exploration of the extension and structure of the island of SHN, in particular for searching for isotopes with longer half-lives predicted to be located in the south east of the island, for new elements, and last not least, for surprises which, naturally, emerge unexpectedly.

  4. TOPICAL REVIEW: Shapes and collectivity of exotic nuclei via low-energy Coulomb excitation

    NASA Astrophysics Data System (ADS)

    Görgen, Andreas

    2010-10-01

    The way in which an atomic nucleus responds to excitations, whether by promoting individual nucleons into higher shells or by collective rotation or vibration, reveals many details of the underlying nuclear structure. The response of the nucleus is closely related to its macroscopic shape. Low-energy Coulomb excitation provides a well-understood means of exciting atomic nuclei, allowing the measurement of static and dynamic electromagnetic moments as a probe of the nuclear wavefunctions. Owing to the availability of radioactive heavy-ion beams with energies near the Coulomb barrier, it is now possible to study the shape and collectivity of short-lived nuclei far from β stability (the so-called exotic nuclei), providing a particularly stringent test of modern theoretical nuclear structure models. This review gives an introduction to the experimental techniques related to low-energy Coulomb excitation with radioactive ion beams and summarizes the results that were obtained over the last 10 years for a wide variety of exotic nuclei at various laboratories employing the isotope separation on-line technique.

  5. Superdeformed oblate superheavy nuclei

    SciTech Connect

    Jachimowicz, P.; Kowal, M.; Skalski, J.

    2011-05-15

    We study stability of superdeformed oblate (SDO) superheavy Z{>=}120 nuclei predicted by systematic microscopic-macroscopic calculations in 12D deformation space and confirmed by the Hartree-Fock calculations with the SLy6 force. We include into consideration high-K isomers that very likely form at the SDO shape. Although half-lives T{sub 1/2} < or approx. 10{sup -5} s are calculated or estimated for even-even spin-zero systems, decay hindrances known for high-K isomers suggest that some SDO superheavy nuclei may be detectable by the present experimental technique.

  6. Hadrons in Nuclei

    SciTech Connect

    Mosel, Ulrich

    2004-08-30

    Changes of hadronic properties in dense nuclear matter as predicted by theory have usually been investigated by means of relativistic heavy-ion reactions. In this talk I show that observable consequences of such changes can also be seen in more elementary reactions on nuclei. Particular emphasis is put on a discussion of photonuclear reactions; examples are the dilepton production at {approx_equal} 1 GeV and the hadron production in nuclei at 10-20 GeV photon energies. The observable effects are expected to be as large as in relativistic heavy-ion collisions and can be more directly related to the underlying hadronic changes.

  7. Quark structure of nuclei

    SciTech Connect

    Blankenbecler, R.

    1981-01-01

    A brief review is given of selected topics involved in the relativistic quark structure of nuclei such as the infinite momentum variables, scaling variables, counting rules, forward-backward variables, thermodynamic-like limit, QCD effects, higher quark bags, confinement, and many unanswered questions.

  8. Transfer involving deformed nuclei

    SciTech Connect

    Rasmussen, J.O.; Guidry, M.W.; Canto, L.F.

    1985-03-01

    Results are reviewed of 1- and 2-neutron transfer reactions at near-barrier energies for deformed nuclei. Rotational angular momentum and excitation patterns are examined. A strong tendency to populating high spin states within a few MeV of the yrast line is noted, and it is interpreted as preferential transfer to rotation-aligned states. 16 refs., 12 figs.

  9. Physics with Polarized Nuclei.

    ERIC Educational Resources Information Center

    Thompson, William J.; Clegg, Thomas B.

    1979-01-01

    Discusses recent advances in polarization techniques, specifically those dealing with polarization of atomic nuclei, and how polarized beams and targets are produced. These techniques have greatly increased the scope of possible studies, and provided the tools for testing fundamental symmetries and the spin dependence of nuclear forces. (GA)

  10. Octupole collectivity in nuclei

    NASA Astrophysics Data System (ADS)

    Butler, P. A.

    2016-07-01

    The experimental and theoretical evidence for octupole collectivity in nuclei is reviewed. Recent theoretical advances, covering a wide spectrum from mean-field theory to algebraic and cluster approaches, are discussed. The status of experimental data on the behaviour of energy levels and electric dipole and electric octupole transition moments is reviewed. Finally, an outlook is given on future prospects for this field.

  11. The decay of hot nuclei

    SciTech Connect

    Moretto, L.G.; Wozniak, G.J.

    1988-11-01

    The formation of hot compound nuclei in intermediate-energy heavy ion reactions is discussed. The statistical decay of such compound nuclei is responsible for the abundant emission of complex fragments and high energy gamma rays. 43 refs., 23 figs.

  12. Energetic Nuclei, Superdensity and Biomedicine

    ERIC Educational Resources Information Center

    Baldin, A. M.

    1977-01-01

    High-energy, relativistic nuclei were first observed in cosmic rays. Studing these nuclei has provided an opportunity for analyzing the composition of cosmic rays and for experimentally verifying principles governing the behavior of nuclear matter at high and super-high temperatures. Medical research using accelerated nuclei is suggested.…

  13. Space Shuttle ice nuclei

    NASA Technical Reports Server (NTRS)

    Turco, R. P.; Toon, O. B.; Whitten, R. C.; Cicerone, R. J.

    1982-01-01

    Estimates are made showing that, as a consequence of rocket activity in the earth's upper atmosphere in the Shuttle era, average ice nuclei concentrations in the upper atmosphere could increase by a factor of two, and that an aluminum dust layer weighing up to 1000 tons might eventually form in the lower atmosphere. The concentrations of Space Shuttle ice nuclei (SSIN) in the upper troposphere and lower stratosphere were estimated by taking into account the composition of the particles, the extent of surface poisoning, and the size of the particles. Calculated stratospheric size distributions at 20 km with Space Shuttle particulate injection, calculated SSIN concentrations at 10 and 20 km altitude corresponding to different water vapor/ice supersaturations, and predicted SSIN concentrations in the lower stratosphere and upper troposphere are shown.

  14. Nuclei in Astrophysics

    NASA Astrophysics Data System (ADS)

    Penionzhkevich, Yu. E.

    2016-06-01

    This work is an attempt to present some problems on the evolution of the Universe: the nucleosynthesis and cosmochronology from the standpoint of physics of particles and nuclei, in particular with the use of the latest results, obtained by means of radioactive nuclear beams. The comparison is made between the processes taking place in the Universe and the mechanisms of formation and decay of nuclei, as well as of their interaction at different energies. Examples are given to show the capabilities of nuclearphysics methods for studying cosmic objects and properties of the Universe. The results of investigations in nuclear reactions, induced by radioactive nuclear beams, make it possible to analyze the nucleosynthesis scenario in the region of light elements in a new manner.

  15. Exotic phenomena in nuclei

    NASA Astrophysics Data System (ADS)

    Neff, Thomas; Feldmeier, Hans; Roth, Robert

    2006-10-01

    In the Fermionic Molecular Dynamics (FMD) model the nuclear many-body system is described using Slater determinants with Gaussian wave-packets as single-particle states. The flexibility of the FMD wave functions allows for a consistent description of shell model like structures, deformed states, cluster structures as well as halos. An effective interaction derived from the realistic Argonne V18 interaction using the Unitary Correlation Operator Method is used for all nuclei. Results for nuclei in the p-shell will be presented. Halo features are present in the Helium isotopes, cluster structures are studied in Beryllium and Carbon isotopes. The interplay between shell structure and cluster structures in the ground and the Hoyle state in ^12C will be discussed.

  16. Pairing forces in nuclei

    SciTech Connect

    Chasman, R.R.

    1996-12-31

    In this contribution, the author mentions some features of pairing forces that are unique to nuclei and cover some areas of major interest in nuclear structure research, that involve pairing. At the level of most nuclear structure studies, nuclei are treated as consisting of two kinds of fermions (protons and neutrons) in a valence space with rather few levels. These features give rise to unique aspects of pairing forces in nuclei: (1) n-p pairing in T = 0 as well as the usual T = 1 pairing that is characteristic of like fermions; (2) a need to correct pairing calculations for the (1/N) effects that can typically be neglected in superconducting solids. An issue of current concern is the nature of the pairing interaction: several recent studies suggest a need for a density dependent form of the pairing interaction. There is a good deal of feedback between the questions of accurate calculations of pairing interactions and the form and magnitude of the pairing interaction. Finally, the authors discuss some many-body wave functions that are a generalization of the BCS wave function form, and apply them to a calculation of energy level spacings in superdeformed rotational bands.

  17. β-Decay half-lives and nuclear structure of exotic proton-rich waiting point nuclei under rp-process conditions

    NASA Astrophysics Data System (ADS)

    Nabi, Jameel-Un; Böyükata, Mahmut

    2016-03-01

    We investigate even-even nuclei in the A ∼ 70 mass region within the framework of the proton-neutron quasi-particle random phase approximation (pn-QRPA) and the interacting boson model-1 (IBM-1). Our work includes calculation of the energy spectra and the potential energy surfaces V (β , γ) of Zn, Ge, Se, Kr and Sr nuclei with the same proton and neutron number, N = Z. The parametrization of the IBM-1 Hamiltonian was performed for the calculation of the energy levels in the ground state bands. Geometric shape of the nuclei was predicted by plotting the potential energy surfaces V (β , γ) obtained from the IBM-1 Hamiltonian in the classical limit. The pn-QRPA model was later used to compute half-lives of the neutron-deficient nuclei which were found to be in very good agreement with the measured ones. The pn-QRPA model was also used to calculate the Gamow-Teller strength distributions and was found to be in decent agreement with the measured data. We further calculate the electron capture and positron decay rates for these N = Z waiting point (WP) nuclei in the stellar environment employing the pn-QRPA model. For the rp-process conditions, our total weak rates are within a factor two compared with the Skyrme HF +BCS +QRPA calculation. All calculated electron capture rates are comparable to the competing positron decay rates under rp-process conditions. Our study confirms the finding that electron capture rates form an integral part of the weak rates under rp-process conditions and should not be neglected in the nuclear network calculations.

  18. Properties of Cometary Nuclei

    NASA Technical Reports Server (NTRS)

    Rahe, J.; Vanysek, V.; Weissman, P. R.

    1994-01-01

    Active long- and short-period comets contribute about 20 to 30 % of the major impactors on the Earth. Cometary nuclei are irregular bodies, typically a few to ten kilometers in diameter, with masses in the range 10(sup 15) to 10(sup 18) g. The nuclei are composed of an intimate mixture of volatile ices, mostly water ice and hydrocarbon and silicate grains. The composition is the closest to solar composition of any known bodies in the solar system. The nuclei appear to be weakly bonded agglomerations of smaller icy planetesimals, and material strengths estimated from observed tidal disruption events are fairly low, typically 10(sup 2) to 10(sup 4) N m(sup -2). Density estimates range between 0.2 and 1.2 g cm(sup -3) but are very poorly determined, if at all. As comets age they develop nonvolitile crusts on their surfaces which eventually render them inactive, similar in appearance to carbonaceous asteroids. However, dormant comets may continue to show sporadic activity and outbursts for some time before they become truly extinct. The source of the long-period comets is the Oort cloud, a vast spherical cloud of perhaps 10(sup 12) to 10(sup 13) comets surrounding the solar system and extending to interstellar distances. The likely source for short-period comets is the Kuiper belt. a ring of perhaps 10(sup 8) to 10(sup 10) remnant icy planetesimals beyond the orbit of Neptune, though some short-period comets may also be long-period comets from the Oort cloud which have been perturbed into short-period orbits.

  19. Electroproduction of Strange Nuclei

    SciTech Connect

    E.V. Hungerford

    2002-06-01

    The advent of high-energy, CW-beams of electrons now allows electro-production and precision studies of nuclei containing hyperons. Previously, the injection of strangeness into a nucleus was accomplished using secondary beams of mesons, where beam quality and target thickness limited the missing mass resolution. We review here the theoretical description of the (e, e'K+) reaction mechanism, and discuss the first experiment demonstrating that this reaction can be used to precisely study the spectra of light hypernuclei. Future experiments based on similar techniques, are expected to attain even better resolutions and rates.

  20. Total photoabsorption in nuclei

    SciTech Connect

    Bianchi, N.

    1992-06-01

    The Frascati-Genova collaboration proposes to measure the total photonuclear cross section on a wide range of nuclei between 500 MeV and 2 GeV, to obtain informations on the interaction of baryon resonances with nucleons and on the onset of the shadowing effect. The experiment could be performed in the Hall B as soon as the tagging facility will be ready and before the end of the installation of the CLAS spectrometer. The requirements for the photon beam, like maximum energy, intensity and beam definition, are not so strong so that the experiment would also be a good first test of the tagged photon facility.

  1. Quark distributions in nuclei

    SciTech Connect

    Catara, F.; Sambataro, M. Italy Dipartimento di Fisica dell'Universita, 95129 Catania )

    1992-08-01

    By making use of a mapping procedure recently proposed, we construct the nucleon image of the one-body quark density operator in the framework of the nonrelativistic quark model of the nucleons. We evaluate the expectation value of this operator in the ground state of the doubly magic nuclei {sup 4}He, {sup 16}O, and {sup 40}Ca described within the nuclear shell model. We analyze the role of quark exchanges between nucleons. We also investigate the effect on the quark density of short-range correlations in the nuclear wave functions as well as of variations in the nucleon size.

  2. Exotic nuclei in astrophysics

    NASA Astrophysics Data System (ADS)

    Penionzhkevich, Yu. E.

    2012-07-01

    Recently the academic community has marked several anniversaries connected with discoveries that played a significant role in the development of astrophysical investigations. The year 2009 was proclaimed by the United Nations the International Year of Astronomy. This was associated with the 400th anniversary of Galileo Galilei's discovery of the optical telescope, which marked the beginning of regular research in the field of astronomy. An important contribution to not only the development of physics of the microcosm, but also to the understanding of processes occurring in the Universe, was the discovery of the atomic nucleus made by E. Rutherford 100 years ago. Since then the investigations in the fields of physics of particles and atomic nuclei have helped to understand many processes in the microcosm. Exactly 80 years ago, K. Yanski used a radio-telescope in order to receive the radiation from cosmic objects for the first time, and at the present time this research area of physics is the most efficient method for studying the properties of the Universe. Finally, the April 12, 1961 (50 years ago) launching of the first sputnik into space with a human being onboard, the Russian cosmonaut Yuri Gagarin, marked the beginning of exploration of the Universe with the direct participation of man. All these achievements considerably extended our ideas about the Universe. This work is an attempt to present some problems on the evolution of the Universe: the nucleosynthesis and cosmochronology from the standpoint of physics of particles and nuclei, in particular with the use of the latest results, obtained by means of radioactive nuclear beams. The comparison is made between the processes taking place in the Universe and the mechanisms of formation and decay of nuclei, as well as of their interaction at different energies. Examples are given to show the capabilities of nuclear-physics methods for studying cosmic objects and properties of the Universe. The results of

  3. IBA in deformed nuclei

    SciTech Connect

    Casten, R.F.; Warner, D.D.

    1982-01-01

    The structure and characteristic properties and predictions of the IBA in deformed nuclei are reviewed, and compared with experiment, in particular for /sup 168/Er. Overall, excellent agreement, with a minimum of free parameters (in effect, two, neglecting scale factors on energy differences), was obtained. A particularly surprising, and unavoidable, prediction is that of strong ..beta.. ..-->.. ..gamma.. transitions, a feature characteristically absent in the geometrical model, but manifest empirically. Some discrepancies were also noted, principally for the K=4 excitation, and the detailed magnitudes of some specific B(E2) values. Considerable attention is paid to analyzing the structure of the IBA states and their relation to geometric models. The bandmixing formalism was studied to interpret both the aforementioned discrepancies and the origin of the ..beta.. ..-->.. ..gamma.. transitions. The IBA states, extremely complex in the usual SU(5) basis, are transformed to the SU(3) basis, as is the interaction Hamiltonian. The IBA wave functions appear with much simplified structure in this way as does the structure of the associated B(E2) values. The nature of the symmetry breaking of SU(3) for actual deformed nuclei is seen to be predominantly ..delta..K=0 mixing. A modified, and more consistent, formalism for the IBA-1 is introduced which is simpler, has fewer free parameters (in effect, one, neglecting scale factors on energy differences), is in at least as good agreement with experiment as the earlier formalism, contains a special case of the 0(6) limit which corresponds to that known empirically, and appears to have a close relationship to the IBA-2. The new formalism facilitates the construction of contour plots of various observables (e.g., energy or B(E2) ratios) as functions of N and chi/sub Q/ which allow the parameter-free discussion of qualitative trajectories or systematics.

  4. Isolation of nuclei from yeast.

    PubMed

    Bhargava, M M; Halvorson, H O

    1971-05-01

    A method for isolation of nuclei from Saccharomyces cervisiae in high yield is described. The DNA/protein ratio of the isolated nuclei is 10 times higher than that of whole cells. Examination of these nuclei in phase and electron microscopes has shown them to be round bodies having a double membrane, microtubules, and a dark crescent at one end. The optimum conditions for extraction and resolution of histones of these nuclei on acrylamide gels have been investigated. The nuclei have an active RNA polymerase (E.C. 2.7.7.6) and are able to synthesize RNA in vitro. They are also readily stainable with Giemsa's, Feulgen's, and acridine orange methods. PMID:19866769

  5. Quarks in Few Body Nuclei

    NASA Astrophysics Data System (ADS)

    Holt, Roy J.

    2016-03-01

    Electron scattering at very high Bjorken x from hadrons provides an excellent test of models, has an important role in high energy physics, and from nuclei, provides a window into short range correlations. Light nuclei have a key role because of the relatively well-known nuclear structure. The development of a novel tritium target for Jefferson Lab has led to renewed interest in the mass three system. For example, deep inelastic scattering experiments in the light nuclei provide a powerful means to determine the neutron structure function. The isospin dependence of electron scattering from mass-3 nuclei provide information on short range correlations in nuclei. The program using the new tritium target will be presented along with a summary of other experiments aimed at revealing the large-x structure of the nucleon.

  6. EVOLUTION OF THE SOLAR NEBULA. IX. GRADIENTS IN THE SPATIAL HETEROGENEITY OF THE SHORT-LIVED RADIOISOTOPES {sup 60}Fe AND {sup 26}Al AND THE STABLE OXYGEN ISOTOPES

    SciTech Connect

    Boss, Alan P.

    2011-10-01

    Short-lived radioisotopes (SLRIs) such as {sup 60}Fe and {sup 26}Al were likely injected into the solar nebula in a spatially and temporally heterogeneous manner. Marginally gravitationally unstable (MGU) disks, of the type required to form gas giant planets, are capable of rapid homogenization of isotopic heterogeneity as well as of rapid radial transport of dust grains and gases throughout a protoplanetary disk. Two different types of new models of an MGU disk in orbit around a solar-mass protostar are presented. The first set has variations in the number of terms in the spherical harmonic solution for the gravitational potential, effectively studying the effect of varying the spatial resolution of the gravitational torques responsible for MGU disk evolution. The second set explores the effects of varying the initial minimum value of the Toomre Q stability parameter, from values of 1.4 to 2.5, i.e., toward increasingly less unstable disks. The new models show that the basic results are largely independent of both sets of variations. MGU disk models robustly result in rapid mixing of initially highly heterogeneous distributions of SLRIs to levels of {approx}10% in both the inner (<5 AU) and outer (>10 AU) disk regions, and to even lower levels ({approx}2%) in intermediate regions, where gravitational torques are most effective at mixing. These gradients should have cosmochemical implications for the distribution of SLRIs and stable oxygen isotopes contained in planetesimals (e.g., comets) formed in the giant planet region ({approx}5 to {approx}10 AU) compared to those formed elsewhere.

  7. Extended Locus of Regular Nuclei

    SciTech Connect

    Amon, L.; Casten, R. F.

    2007-04-23

    A new family of IBM Hamiltonians, characterized by certain parameter values, was found about 15 years ago by Alhassid and Whelan to display almost regular dynamics, and yet these solutions to the IBM do not belong to any of the known dynamical symmetry limits (vibrational, rotational and {gamma} - unstable). Rather, they comprise an 'Arc of Regularity' cutting through the interior of the symmetry triangle from U(5) to SU(3) where suddenly there is a decrease in chaoticity and a significant increase in regularity. A few years ago, the first set of nuclei lying along this arc was discovered. The purpose of the present work is to search more broadly in the nuclear chart at all nuclei from Z = 40 - 100 for other examples of such 'regular' nuclei. Using a unique signature for such nuclei involving energy differences of certain excited states, we have identified an additional set of 12 nuclei lying near or along the arc. Some of these nuclei are known to have low-lying intruder states and therefore care must be taken, however, in judging their structure. The regularity exhibited by nuclei near the arc presumably reflects the validity or partial validity of some new, as yet unknown, quantum number describing these systems and giving the regularity found for them.

  8. Shape coexistence in atomic nuclei

    SciTech Connect

    Heyde, Kris; Wood, John L.

    2011-10-01

    Shape coexistence in nuclei appears to be unique in the realm of finite many-body quantum systems. It differs from the various geometrical arrangements that sometimes occur in a molecule in that in a molecule the various arrangements are of the widely separated atomic nuclei. In nuclei the various ''arrangements'' of nucleons involve (sets of) energy eigenstates with different electric quadrupole properties such as moments and transition rates, and different distributions of proton pairs and neutron pairs with respect to their Fermi energies. Sometimes two such structures will ''invert'' as a function of the nucleon number, resulting in a sudden and dramatic change in ground-state properties in neighboring isotopes and isotones. In the first part of this review the theoretical status of coexistence in nuclei is summarized. Two approaches, namely, microscopic shell-model descriptions and mean-field descriptions, are emphasized. The second part of this review presents systematic data, for both even- and odd-mass nuclei, selected to illustrate the various ways in which coexistence is observed in nuclei. The last part of this review looks to future developments and the issue of the universality of coexistence in nuclei. Surprises continue to be discovered. With the major advances in reaching to extremes of proton-neutron number, and the anticipated new ''rare isotope beam'' facilities, guidelines for search and discovery are discussed.

  9. Gluon density in nuclei

    SciTech Connect

    Ayala, A.L.; Ducati, M.B.G.; Levin, E.M.

    1996-10-01

    In this talk we present our detailed study (theory and numbers) on the shadowing corrections to the gluon structure functions for nuclei. Starting from rather controversial information on the nucleon structure function which is originated by the recent HERA data, we develop the Glauber approach for the gluon density in a nucleus based on Mueller formula and estimate the value of the shadowing corrections in this case. Then we calculate the first corrections to the Glauber approach and show that these corrections are big. Based on this practical observation we suggest the new evolution equation which takes into account the shadowing corrections and solve it. We hope to convince you that the new evolution equation gives a good theoretical tool to treat the shadowing corrections for the gluons density in a nucleus and, therefore, it is able to provide the theoretically reliable initial conditions for the time evolution of the nucleus-nucleus cascade. The initial conditions should be fixed both theoretically and phenomenologically before to attack such complicated problems as the mixture of hard and soft processes in nucleus-nucleus interactions at high energy or the theoretically reliable approach to hadron or/and parton cascades for high energy nucleus-nucleus interaction. 35 refs., 24 figs., 1 tab.

  10. Stem cell mechanics: Auxetic nuclei

    NASA Astrophysics Data System (ADS)

    Wang, Ning

    2014-06-01

    The nuclei of naive mouse embryonic stem cells that are transitioning towards differentiation expand when the cells are stretched and contract when they are compressed. What drives this auxetic phenotype is, however, unclear.

  11. Alpha Condensates in Atomic Nuclei

    SciTech Connect

    Suzuki, Y.; Matsumura, H.

    2005-11-21

    Recent issues on Bose-Einstein condensation (BEC) of {alpha}-particles in nuclei are reviewed. A candidate of condensates is discussed for some states in 12C and 16O by defining the amount of {alpha} condensation.

  12. Generalized parton distributions in nuclei

    SciTech Connect

    Vadim Guzey

    2009-12-01

    Generalized parton distributions (GPDs) of nuclei describe the distribution of quarks and gluons in nuclei probed in hard exclusive reactions, such as e.g. deeply virtual Compton scattering (DVCS). Nuclear GPDs and nuclear DVCS allow us to study new aspects of many traditional nuclear effects (nuclear shadowing, EMC effect, medium modifications of the bound nucleons) as well as to access novel nuclear effects. In my talk, I review recent theoretical progress in the area of nuclear GPDs.

  13. The nature of comet nuclei

    NASA Technical Reports Server (NTRS)

    Sykes, Mark V.; Walker, Russell G.

    1992-01-01

    The icy-conglomerate model of comet nuclei has dominated all others since its introduction. It provided a basis for understanding the non-gravitational motions of comets which had perplexed dynamicists up to that time, and provided a focus for understanding cometary composition and origin. The image of comets as dirty snowballs was quickly adopted. Comet nuclei including their trail mass loss rates and refractory to volatile mass ratios are described.

  14. Study of short-lived climate forcers atmospheric variability at Kathmandu and at the WMO/GAW Global Station "Nepal Climate Observatory-Pyramid" (5079 m a.s.l.) in the Himalayas

    NASA Astrophysics Data System (ADS)

    Putero, Davide; Cristofanelli, Paolo; Adhikary, Bhupesh; Marinoni, Angela; Duchi, Rocco; Calzolari, Francescopiero; Landi, Tony Christian; Pietro Verza, Gian; Alborghetti, Marcello; Vuillermoz, Elisa; Rupakheti, Maheswar; Lawrence, Mark; Bonasoni, Paolo

    2014-05-01

    Aerosols and tropospheric ozone play a key role in the climate system, since they are short-lived climate forcers (SLCFs). South Asia represents a "hot-spot" in terms of climate change, since a vast region extending from the Indian Ocean to the Himalayas appears to be affected by large amounts of aerosols and pollutant gases (the so-called Atmospheric Brown Cloud). In the framework of the SusKat - ABC field campaign, a new measurement station has been installed in Pakanajol, Kathmandu (Nepal) on January 2013. This station is representative of the severe polluted conditions of the Kathmandu valley. Continuous measurements of equivalent black carbon (eqBC), surface ozone (O3), aerosol number concentration and size distribution, on-line PM10-PM1, as well as meteorological parameters, are carried out at this sampling site. In the high Himalayas (150 km north-east from Kathmandu), continuous atmospheric composition measurements are performed at the WMO/GAW Global Station Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.) in the Southern Himalayas. This measurement site is representative of the background conditions of the Himalayan ridge and measurements of eqBC, O3, aerosol number size distribution and meteorological parameters are continuously carried out since March 2006. The aim of this work is to compare the variability of atmospheric composition between the two sampling sites, with a particular emphasis on SLCFs, thus providing two complementary perspectives about the Atmospheric Brown Cloud phenomenon. Moreover, hints about the possible role of vertical air-mass transport of SLCFs from the foothills to the high Himalayas will be provided. The seasonal trend of eqBC at Pakanajol is characterized by a decreasing behavior from winter to monsoon, while at NCO-P it is characterized by a clear pre-monsoon maximum. On the other hand, at both sampling sites, O3 and particle number (accumulation and coarse) showed highest values during the pre-monsoon (April

  15. Extracting nuclear sizes of medium to heavy nuclei from total reaction cross sections

    NASA Astrophysics Data System (ADS)

    Horiuchi, W.; Hatakeyama, S.; Ebata, S.; Suzuki, Y.

    2016-04-01

    Background: Proton and neutron radii are fundamental quantities of atomic nuclei. To study the sizes of short-lived unstable nuclei, there is a need for an alternative to electron scattering. Purpose: The recent paper by Horiuchi et al. [Phys. Rev. C 89, 011601(R) (2014)], 10.1103/PhysRevC.89.011601 proposed a possible way of extracting the matter and neutron-skin thickness of light- to medium-mass nuclei using total reaction cross section, σR. The analysis is extended to medium to heavy nuclei up to lead isotopes with due attention to Coulomb breakup contributions as well as density distributions improved by paring correlation. Methods: We formulate a quantitative calculation of σR based on the Glauber model including the Coulomb breakup. To substantiate the treatment of the Coulomb breakup, we also evaluate the Coulomb breakup cross section due to the electric dipole field in a canonical-basis-time-dependent-Hartree-Fock-Bogoliubov theory in the three-dimensional coordinate space. Results: We analyze σR's of 103 nuclei with Z =20 , 28, 40, 50, 70, and 82 incident on light targets, H,21, 4He, and 12C. Three kinds of Skyrme interactions are tested to generate those wave functions. To discuss possible uncertainty due to the Coulomb breakup, we examine its dependence on the target, the incident energy, and the Skyrme interaction. The proton is a most promising target for extracting the nuclear sizes as the Coulomb excitation can safely be neglected. We find that the so-called reaction radius, aR=√{σR/π } , for the proton target is very well approximated by a linear function of two variables, the matter radius and the skin thickness, in which three constants depend only on the incident energy. We quantify the accuracy of σR measurements needed to extract the nuclear sizes. Conclusions: The proton is the best target because, once the incident energy is set, its aR is very accurately determined by only the matter radius and neutron-skin thickness. If σR's at

  16. Nuclear-physics characteristics of short-lived odd-odd {sup 232}Pa, {sup 238}Np and {sup 242g}Am nuclides (measurement results and prospects for further researches)

    SciTech Connect

    Fomushkin, Eduard F.; Abramovich, Sergei N.; Andreev, Mikhail F.

    1998-10-26

    In VNIIEF there were measured cross-sections of {sup 232}Pa and {sup 238}Np fission caused by thermal neutrons. The obtained data do not agree with the results of measurements carried out in Los Alamos National Laboratory (USA). Possible reasons of the result divergence are discussed. There are considered the measurement prospects for fission and radiation capture cross-sections of thermal neutrons by the nuclei of {sup 232}Pa, {sup 238}Np and {sup 242g}Am, including the measurements performed with the aid of ILL (Grenoble, France) reactor and some devices for neutron researches.

  17. Cavitation inception from bubble nuclei.

    PubMed

    Mørch, K A

    2015-10-01

    The tensile strength of ordinary water such as tap water or seawater is typically well below 1 bar. It is governed by cavitation nuclei in the water, not by the tensile strength of the water itself, which is extremely high. Different models of the nuclei have been suggested over the years, and experimental investigations of bubbles and cavitation inception have been presented. These results suggest that cavitation nuclei in equilibrium are gaseous voids in the water, stabilized by a skin which allows diffusion balance between gas inside the void and gas in solution in the surrounding liquid. The cavitation nuclei may be free gas bubbles in the bulk of water, or interfacial gaseous voids located on the surface of particles in the water, or on bounding walls. The tensile strength of these nuclei depends not only on the water quality but also on the pressure-time history of the water. A recent model and associated experiments throw new light on the effects of transient pressures on the tensile strength of water, which may be notably reduced or increased by such pressure changes. PMID:26442138

  18. Polarized EMC Effect in Nuclei

    SciTech Connect

    Ian Cloet; A. W. Thomas; W. Bentz

    2006-06-05

    The discovery of the EMC effect and the proton spin crisis by the European Muon Collaboration are two of the standout experiments of the last 25 years. It is therefore surprising that there has been no experimental and little theoretical investigation of the spin structure functions of atomic nuclei. To address this we present results for the spin-dependent structure functions of nuclei. The quark degrees of freedom in nuclei are accessed via the convolution formalism. Where the nucleon bound state is obtained by solving the relativistic Faddeev equation, and a relativistic shell model is used to model the atomic nucleus. We find the important result that the medium modifications to the polarized structure functions are about twice that of the unpolarized case.

  19. A multi-model intercomparison of halogenated very short-lived substances (TransCom-VSLS): linking oceanic emissions and tropospheric transport for a reconciled estimate of the stratospheric source gas injection of bromine

    NASA Astrophysics Data System (ADS)

    Hossaini, R.; Patra, P. K.; Leeson, A. A.; Krysztofiak, G.; Abraham, N. L.; Andrews, S. J.; Archibald, A. T.; Aschmann, J.; Atlas, E. L.; Belikov, D. A.; Bönisch, H.; Carpenter, L. J.; Dhomse, S.; Dorf, M.; Engel, A.; Feng, W.; Fuhlbrügge, S.; Griffiths, P. T.; Harris, N. R. P.; Hommel, R.; Keber, T.; Krüger, K.; Lennartz, S. T.; Maksyutov, S.; Mantle, H.; Mills, G. P.; Miller, B.; Montzka, S. A.; Moore, F.; Navarro, M. A.; Oram, D. E.; Pfeilsticker, K.; Pyle, J. A.; Quack, B.; Robinson, A. D.; Saikawa, E.; Saiz-Lopez, A.; Sala, S.; Sinnhuber, B.-M.; Taguchi, S.; Tegtmeier, S.; Lidster, R. T.; Wilson, C.; Ziska, F.

    2016-07-01

    The first concerted multi-model intercomparison of halogenated very short-lived substances (VSLS) has been performed, within the framework of the ongoing Atmospheric Tracer Transport Model Intercomparison Project (TransCom). Eleven global models or model variants participated (nine chemical transport models and two chemistry-climate models) by simulating the major natural bromine VSLS, bromoform (CHBr3) and dibromomethane (CH2Br2), over a 20-year period (1993-2012). Except for three model simulations, all others were driven offline by (or nudged to) reanalysed meteorology. The overarching goal of TransCom-VSLS was to provide a reconciled model estimate of the stratospheric source gas injection (SGI) of bromine from these gases, to constrain the current measurement-derived range, and to investigate inter-model differences due to emissions and transport processes. Models ran with standardised idealised chemistry, to isolate differences due to transport, and we investigated the sensitivity of results to a range of VSLS emission inventories. Models were tested in their ability to reproduce the observed seasonal and spatial distribution of VSLS at the surface, using measurements from NOAA's long-term global monitoring network, and in the tropical troposphere, using recent aircraft measurements - including high-altitude observations from the NASA Global Hawk platform. The models generally capture the observed seasonal cycle of surface CHBr3 and CH2Br2 well, with a strong model-measurement correlation (r ≥ 0.7) at most sites. In a given model, the absolute model-measurement agreement at the surface is highly sensitive to the choice of emissions. Large inter-model differences are apparent when using the same emission inventory, highlighting the challenges faced in evaluating such inventories at the global scale. Across the ensemble, most consistency is found within the tropics where most of the models (8 out of 11) achieve best agreement to surface CHBr3 observations

  20. Level densities of heaviest nuclei

    NASA Astrophysics Data System (ADS)

    Bezbakh, A. N.; Shneidman, T. M.; Adamian, G. G.; Antonenko, N. V.

    2014-06-01

    The intrinsic level densities of superheavy nuclei in the α-decay chains of 296,298,300120 are calculated using the single-particle spectra obtained with the modified two-center shell model. The role of the shell and pairing effects on the level density as well as their quenching with excitation energy are studied. The extracted level density parameter is expressed as a function of mass number, ground-state shell correction, and excitation energy. The results are compared with the phenomenological values of level density parameters used to calculate the survival of excited heavy nuclei.

  1. Colored models for anomalous nuclei

    SciTech Connect

    Watson, P.J.S.; Saly, R.; Romo, W.J.; Sundaresan, M.K.; Campbell, B.; Elias, V.

    1983-04-01

    There seems to be good experimental evidence that anomalous nuclei are produced in heavy-ion collisions; they are anomalous in that they have an abnormally short mean free path, for example, in nuclear emulsions. Here we consider the possibility that anomalous nuclei are combinations of a colored anomalous particle fragment (based on theories with spontaneous breakdown of color symmetry) with ordinary nucleons. Phenomenological implications of various possible models in which the anomalous particle fragment is considered to be a colored particle with the color symmetry SU(3)/sub c/ explicitly broken are given.

  2. Neutron scattering on deformed nuclei

    NASA Astrophysics Data System (ADS)

    Hansen, L. F.; Haight, R. C.; Pohl, B. A.; Wong, C.; Lagrange, Ch.

    1985-01-01

    Measurements of neutron elastic and inelastic differential cross sections around 14 MeV for 9Be, C, 181Ta, 232Th, 238U, and 239Pu have been analyzed using a coupled channel (CC) formalism for deformed nuclei and phenomenological global optical model potentials (OMP). For the actinide targets these results are compared with the predictions of a semi-microscopic calculation using Jeukenne, Lejeune, and Mahaux (JLM) microscopic OMP and a deformed ground state nuclear density. The overall agreement between calculations and the measurements is reasonably good even for the very light nuclei, where the quality of the fits is better than those obtained with spherical OMP.

  3. Octupole shapes in heavy nuclei

    SciTech Connect

    Ahmad, I.

    1994-08-01

    Theoretical calculations and measurements show the presence of strong octupole correlations in thecyround states and low-lying states of odd-mass and odd-odd nuclei in the RaPa region. Evidence for octupole correlations is provided by the observation of parity doublets and reductions in M1 matrix elements, decoupling parameters, and Coriolis matrix elements Involving high-j states. Enhancement of E1 transition rates has also been observed for some of the octupole deformed nuclei. The most convincing argument for octupole deformation is provided by the similarities of the reduced alpha decay rates to the two members of parity doublets.

  4. Exotic nuclei and nuclear forces

    NASA Astrophysics Data System (ADS)

    Otsuka, Takaharu

    2013-01-01

    I overview new aspects of the structure of exotic nuclei as compared to stable nuclei, focusing on several characteristic effects of nuclear forces. The shell structure of nuclei has been proposed by Mayer and Jensen, and has been considered to be kept valid basically for all nuclei, with well-known magic numbers, 2, 8, 20, 28, 50, …. Nuclear forces were shown, very recently, to change this paradigm. It will be presented that the evolution of shell structure occurs in various ways as more neutrons and/or protons are added, and I will present basic points of this shell evolution in terms of the monopole interaction of nuclear forces. I will discuss three types of nuclear forces. The first one is the tensor force. The tensor force is one of the most fundamental nuclear forces, but its first-order effect on the shell structure has been clarified only recently in studies on exotic nuclei. The tensor force can change the spin-orbit splitting depending on the occupation of specific orbits. This results in changes of the shell structure in many nuclei, and consequently some of Mayer-Jensen's magic numbers are lost and new ones emerge, in certain nuclei. This mechanism can be understood in an intuitive way, meaning that the effect is general and robust. The second type of nuclear forces is central force. I will show a general but unknown property of the central force in the shell-model Hamiltonian that can describe nuclear properties in a good agreement with experiment. I will then demonstrate how it can be incorporated into a simple model of the central force, and will discuss how this force works in the shell evolution. Actually, by combining this central force with the tensor force, one can understand and foresee how the same proton-neutron interaction drives the shell evolution, for examples such as Sn/Sb isotopes, N = 20 nuclei and Ni/Cu isotopes. The distribution of single-particle strength is discussed also in comparison to (e,e‧p) experiment on 48Ca. The shell

  5. Electromagnetic structure of light nuclei

    DOE PAGESBeta

    Pastore, Saori

    2016-03-25

    Here, the present understanding of nuclear electromagnetic properties including electromagnetic moments, form factors and transitions in nuclei with A ≤ 10 is reviewed. Emphasis is on calculations based on nuclear Hamiltonians that include two- and three-nucleon realistic potentials, along with one- and two-body electromagnetic currents derived from a chiral effective field theory with pions and nucleons.

  6. Proton Distribution in Heavy Nuclei

    DOE R&D Accomplishments Database

    Johnson, M. H; Teller, E.

    1953-11-13

    It is reasoned that, from considerations connected with beta-decay stability and Coulomb repulsion forces, a neutron excess is developed on the surface of heavy nuclei. Several consequences of this qualitative analysis in nucleon interactions are briefly noted. (K.S.)

  7. Octupole correlation effects in nuclei

    SciTech Connect

    Chasman, R.R.

    1992-08-01

    Octupole correlation effects in nuclei are discussed from the point of view of many-body wavefunctions as well as mean-field methods. The light actinides, where octupole effects are largest, are considered in detail. Comparisons of theory and experiment are made for energy splittings of parity doublets; E1 transition matrix elements and one-nucleon transfer reactions.

  8. Octupole correlation effects in nuclei

    SciTech Connect

    Chasman, R.R.

    1992-01-01

    Octupole correlation effects in nuclei are discussed from the point of view of many-body wavefunctions as well as mean-field methods. The light actinides, where octupole effects are largest, are considered in detail. Comparisons of theory and experiment are made for energy splittings of parity doublets; E1 transition matrix elements and one-nucleon transfer reactions.

  9. Transitional nuclei near shell closures

    SciTech Connect

    Mukherjee, G.

    2014-08-14

    High spin states in Bismuth and Thallium nuclei near the Z = 82 shell closure and Cesium nuclei near the N = 82 shell closure in A = 190 and A = 130 regions, respectively, have been experimentally investigated using heavy-ion fusion evaporation reaction and by detecting the gamma rays using the Indian National Gamma Array (INGA). Interesting shape properties in these transitional nuclei have been observed. The results were compared with the neighboring nuclei in these two regions. The total Routhian surface (TRS) calculations have been performed for a better understanding of the observed properties. In mass region A = 190, a change in shape from spherical to deformed has been observd around neutron number N = 112 for the Bi (Z = 83) isotopes with proton number above the magic gap Z = 82, whereas, the shape of Tl (Z = 81) isotopes with proton number below the magic gap Z = 82 remains stable as a function of neutron number. An important transition from aplanar to planar configuration of angular momentum vectors leading to the occurance of nuclar chirality and magnetic rotation, respectively, has been proposed for the unique parity πh{sub 11/2}⊗νh{sub 11/2} configuration in Cs isotopes in the mass region A ∼ 130 around neutron number N = 79. These results are in commensurate with the TRS calculations.

  10. International Symposium on Exotic Nuclei

    NASA Astrophysics Data System (ADS)

    Penionzhkevich, Yu. E.; Cherepanov, E. A.

    Methods of production of light exotic nuclei and study of their ptoperties -- Superheavy elements. Syhnthesis and properties -- Nuclear fission -- Nuclear reactions -- rare processes, decay and nuclear structure -- Experimental set-ups and future projects -- Radioactive beams. Production and research programmes -- Public relations.

  11. CLOUD CONDENSATION NUCLEI MEASUREMENTS WITHIN CLOUDS

    EPA Science Inventory

    Measurements of the spectra of cloud condensation nuclei (CCN) within and near the boundaries of clouds are presented. Some of the in-cloud measurements excluded the nuclei within cloud droplets (interstitial CCN) while others included all nuclei inside the cloud (total CCN). The...

  12. Large-scale evaluation of β -decay rates of r -process nuclei with the inclusion of first-forbidden transitions

    NASA Astrophysics Data System (ADS)

    Marketin, T.; Huther, L.; Martínez-Pinedo, G.

    2016-02-01

    Background: r -process nucleosynthesis models rely, by necessity, on nuclear structure models for input. Particularly important are β -decay half-lives of neutron-rich nuclei. At present only a single systematic calculation exists that provides values for all relevant nuclei making it difficult to test the sensitivity of nucleosynthesis models to this input. Additionally, even though there are indications that their contribution may be significant, the impact of first-forbidden transitions on decay rates has not been systematically studied within a consistent model. Purpose: Our goal is to provide a table of β -decay half-lives and β -delayed neutron emission probabilities, including first-forbidden transitions, calculated within a fully self-consistent microscopic theoretical framework. The results are used in an r -process nucleosynthesis calculation to asses the sensitivity of heavy element nucleosynthesis to weak interaction reaction rates. Method: We use a fully self-consistent covariant density functional theory (CDFT) framework. The ground state of all nuclei is calculated with the relativistic Hartree-Bogoliubov (RHB) model, and excited states are obtained within the proton-neutron relativistic quasiparticle random phase approximation (p n -RQRPA). Results: The β -decay half-lives, β -delayed neutron emission probabilities, and the average number of emitted neutrons have been calculated for 5409 nuclei in the neutron-rich region of the nuclear chart. We observe a significant contribution of the first-forbidden transitions to the total decay rate in nuclei far from the valley of stability. The experimental half-lives are in general well reproduced for even-even, odd-A , and odd-odd nuclei, in particular for short-lived nuclei. The resulting data table is included with the article as Supplemental Material. Conclusions: In certain regions of the nuclear chart, first-forbidden transitions constitute a large fraction of the total decay rate and must be

  13. Pairing in hot rotating nuclei

    SciTech Connect

    Hung, N. Quang; Dang, N. Dinh

    2008-12-15

    Nuclear pairing properties are studied within an approach that includes the quasiparticle-number fluctuation (QNF) and coupling to the quasiparticle-pair vibrations at finite temperature and angular momentum. The formalism is developed to describe noncollective rotations about the symmetry axis. The numerical calculations are performed within a doubly folded equidistant multilevel model as well as several realistic nuclei. The results obtained for the pairing gap, total energy, and heat capacity show that the QNF smoothes out the sharp SN phase transition and leads to the appearance of a thermally assisted pairing gap in rotating nuclei at finite temperature. The corrections due to the dynamic coupling to SCQRPA vibrations and particle-number projection are analyzed. The effect of backbending of the momentum of inertia as a function of squared angular velocity is also discussed.

  14. Superheavy nuclei and fission barriers

    NASA Astrophysics Data System (ADS)

    Lu, Bing-Nan; Zhao, Jie; Zhao, En-Guang; Zhou, Shan-Gui

    In this chapter, we will present relativistic mean field (RMF) description of heavy and superheavy nuclei (SHN). We will discuss the shell structure and magic numbers in the mass region of SHN, binding energies and α decay Q values, shapes of ground states and potential energy surfaces and fission barriers. We particularly focus on the multidimensionally-constrained covariant density functional theories (CDFT) and the applications of CDFT to the study of exotic nuclear shapes and fission barriers.

  15. Direct Reactions with Exotic Nuclei

    SciTech Connect

    Baur, G.; Typel, S.

    2005-10-14

    We discuss recent work on Coulomb dissociation and an effective-range theory of low-lying electromagnetic strength of halo nuclei. We propose to study Coulomb dissociation of a halo nucleus bound by a zero-range potential as a homework problem. We study the transition from stripping to bound and unbound states and point out in this context that the Trojan-Horse method is a suitable tool to investigate subthreshold resonances.

  16. PREFACE: Correlation Dynamics in Nuclei

    NASA Astrophysics Data System (ADS)

    Suzuki, Toshio; Otsuka, Takaharu; Ichimura, Munetake

    2005-01-01

    The International Symposium on `Correlation Dynamics in Nuclei' was held at the Sanjo Kaikan, the University of Tokyo, from the 31 January to 4 February 2005. This symposium was organized on the occasion of the 50th anniversary of the Configuration Mixing theory of Arima and Horie. The symposium was hosted by the University of Tokyo, and supported by the Inoue Foundation for Science, the Japan Atomic Energy Research Institute and the Ministry of Education, Culture, Sports, Science and Technology. The purpose of the symposium was to discuss theoretical and experimental developments and future prospects in physics of correlation dynamics in nuclei, including topics such as effective interactions, shell model studies of configuration mixing and spin-isospin modes in nuclei. It was shown in many ways and angles that the Arima-Horie theory has been a starting point of a variety of developments of the studies in these fields over many decades. The developments have been enhanced by the expansion of computational capabilities and the progress in accelerators, detectors and radioactive beam facilities. We enjoyed 28 excellent and lively invited talks and 30 oral presentations in the symposium with about 90 participants. A special session was dedicated to celebrate the 80th birthday of Professor Igal Talmi, who made invaluable and pioneering works in the shell model theory. Finally, we would like to thank all the speakers and the participants as well as the other organizers for their contributions which made the symposium very successful.

  17. NUCLEI AT HIGH ANGULAR MOMENTUM

    SciTech Connect

    Diamond, R.M.; Stephens, F.S.

    1980-06-01

    It appears that most nuclei show a compromise between purely collective and purely non-collective behavior at very high spins.non~collective behavior in nuclei has been seen only as high as 36 or 37{bar h}, at which point a more collective structure seems to develop. The concepts underlying the study of high angular momentum states are discussed. The factors that limit angular momentum in nuclei are considered. The currently emerging state of physics of very high spin states is reviewed. The detailed calculations currently made for high spin states are described, focusing not on the calculations themselves, but on the physical input to them and results that come out. Production of high-spin states using heavy-ion reactions is reviewed. Studies of {gamma}-rays de-exciting the evaporation residues from heavy-ion reactions are covered. Two types of {gamma} rays occur: those that cool the nucleus to or toward the yrast line, called "statistical," and those that are more or less parallel to the yrast line and remove the angular momentum, called "yrast~like." Collective rotation, in simplest form the motion of a deformed nucleus around an axis perpendicular to its symmetry axis, is also covered.

  18. Structure functions for light nuclei

    SciTech Connect

    S.A. Kulagin, R. Petti

    2010-11-01

    We discuss the nuclear EMC effect with particular emphasis on recent data for light nuclei including 2H, 3He, 4He, 9Be, 12C and 14N. In order to verify the consistency of available data, we calculate the \\chi^2 deviation between different data sets. We find a good agreement between the results from the NMC, SLAC E139, and HERMES experiments. However, our analysis indicates an overall normalization offset of about 2% in the data from the recent JLab E03-103 experiment with respect to previous data for nuclei heavier than 3He. We also discuss the extraction of the neutron/proton structure function ratio F2n/F2p from the nuclear ratios 3He/2H and 2H/1H. Our analysis shows that the E03-103 data on 3He/2H require a renormalization of about 3% in order to be consistent with the F2n/F2p ratio obtained from the NMC experiment. After such a renormalization, the 3He data from the E03-103 data and HERMES experiments are in a good agreement. Finally, we present a detailed comparison between data and model calculations, which include a description of the nuclear binding, Fermi motion and off-shell corrections to the structure functions of bound proton and neutron, as well as the nuclear pion and shadowing corrections. Overall, a good agreement with the available data for all nuclei is obtained.

  19. Isomer Studies for Nuclei near the Proton Drip Line in the Mass 130-160 Region

    SciTech Connect

    Cullen, D. M.; Mason, P. J. R.; Khan, S.; Kishada, A. M.; Varley, B. J.; Rigby, S. V.; Scholey, C.; Greenlees, P.; Rahkila, P.; Jones, P. M.; Julin, R.; Juutinen, S.; Leino, M.; Leppaenen, A. P.; Nyman, M.; Uusitalo, J.; Grahn, T.; Nieminen, P.; Pakarinen, J.

    2007-11-30

    This report details the status of an experimental research programme which has studied isomeric states in the mass 130-160 region of the nuclear chart. Several new isomers have been established and characterised near the proton drip line using a recoil isomer tagging technique at the University of Jyvaeskylae, Finland. The latest experiments have been performed with a modified setup where the standard GREAT focal-plane double-sided silicon-strip detector was changed to a dual multi-wire proportional-counter arrangement. This new setup has improved capability for short-lived isomer studies where high focal-plane rates can be tolerated. The results of key recent experiments for nuclei situated above ({sup 153}Yb,{sup 152}Tm) and below ({sup 136}Pm,{sup 142}Tb) the N = 82 shell gap were presented along with an interpretation for the isomers. Finally, the future prospects of the technique, using an isomer-tagged differential-plunger setup, were discussed. This technique will be capable of establishing the deformation of the states above the isomers and will aid in the process of assigning underlying single-particle configurations to the isomeric states.

  20. Physical characteristics of mouse sperm nuclei.

    PubMed Central

    Wyrobek, A J; Meistrich, M L; Furrer, R; Bruce, W R

    1976-01-01

    The nuclei of epididymal sperm, isolated from C57BL/6J and CBA/J inbred mice by their resistance to trypsin digestion, retain the shape differences of the intact sperm head. Various physical characteristics of these nuclei were measured and compared. The measurement of the projected dimensions of nuclei showed that the CBA nuclei are 13.5% longer than C57BL/6 nuclei (8.64 +/- 0.02 mum compared with 7.61 +/- 0.02 mum), 0.8% narrower (3.51 +/- 0.01 vs. 3.54 +/-0.01 mum) with 6.8% more area (22.34 +/- 0.10 vs. 20.91 +/- 0.09 mum2). However, the volumes of the nuclei as based on reconstructing calibrated electronmicrographs of serial sections of the nuclei indicated that CBA are about 7% smaller than C57BL/6 nuclei (3.72 +/- 0.08 vs. 4.01 +/- 0.03 mum3). The buoyant density of the CBA nuclei is 1.435 +/- 0.002 g/cm3 compared with 1.433 +/- 0.002 g/cm3 for the C57BL/6 nuclei as determined on linear CsCl and Renografin-76 density gradients and confirmed by a technique utilizing physiological tonicities. Therefore, the average mass of the CBA nuclei is less than that of the C57BL/6 nuclei (5.34 +/- 0.12 vs. 5.75 +/- 0.05 pg). The sedimentation velocities at unit gravity of nuclei from 11 inbred strains differ over a range of more than 6% with CBA nuclei sedimenting about 2.0% more slowly than C57BL/6 nuclei. We show that for these nuclei the sedimentation velocity can be related to their buoyant density, volume and a sedimentation shape factor. Within the errors of our measurements of these various characteristics, it was found that C57BL/6 and CBA nuclei have similar sedimentation shape factors. Therefore, the difference in sedimentation velocity between these nuclei appears to be primarily a result of differences in volume. The possible applications of these techniques to the physical separation of sperm are evaluated in the discussion. Images FIGURE 1 PMID:938720

  1. Structure functions for light nuclei

    SciTech Connect

    Kulagin, S. A.; Petti, R.

    2010-11-15

    We discuss the nuclear EMC effect with particular emphasis on recent data for light nuclei including {sup 2}H, {sup 3}He, {sup 4}He, {sup 9}Be, {sup 12}C, and {sup 14}N. In order to verify the consistency of available data, we calculate the {chi}{sup 2} deviation between different data sets. We find a good agreement between the results from the NMC, SLAC E139, and HERMES experiments. However, our analysis indicates an overall normalization offset of about 2% in the data from the recent JLab E03-103 experiment with respect to previous data for nuclei heavier than {sup 3}He. We also discuss the extraction of the neutron/proton structure function ratio F{sub 2}{sup n}/F{sub 2}{sup p} from the nuclear ratios {sup 3}He/{sup 2}H and {sup 2}H/{sup 1}H. Our analysis shows that the E03-103 data on {sup 3}He/{sup 2}H require a renormalization of about 3% in order to be consistent with the F{sub 2}{sup n}/F{sub 2}{sup p} ratio obtained from the NMC experiment. After such a renormalization, the {sup 3}He data from the E03-103 and HERMES experiments are in a good agreement. Finally, we present a detailed comparison between data and model calculations, which include a description of the nuclear binding, Fermi motion, and off-shell corrections to the structure functions of bound proton and neutron, as well as the nuclear pion and shadowing corrections. Overall, a good agreement with the available data for all nuclei is obtained.

  2. The rotation of comet nuclei

    NASA Technical Reports Server (NTRS)

    Whipple, F. L.

    1982-01-01

    Spin-vector research on cometary nuclei is reviewed with emphasis on the actual determination of rotation period and spin-axis orientation. The rotation periods of 47 comets are compared with those of 41 asteroids with diameters of not more than 40 km. It is shown that the median periods for the comets is 15.0 hr as compared with 6.8 hr for the asteroids and that the preliminary distribution curve for the logarithms of the comet periods is not Gaussian and is flatter than the corresponding curve for the asteroids. Slow accumulation at low relative velocities is suggested as the cause of the longer comet rotation periods.

  3. Short Range Correlations in Nuclei

    SciTech Connect

    L. B. Weinstein

    2006-11-01

    Short range correlations (SRC) are an extremely important part of nuclear structure. They are responsible for the high momentum part of the nuclear wavefunction. Instantaneous densities can significantly exceed the average neutron star density. Recent (e,e[prime]) measurements at Jefferson Lab have shown that SRC are universal in nuclei from deuterium to gold, that the probability of two-nucleon SRC is 5-25%, and that the probability of three-nucleon SRC is less than 1%. Recent (e,e[prime]pn) measurements have measured the SRC probabilities as a function of proton momentum and have measured the joint NN momentum distributions.

  4. Review of metastable states in heavy nuclei.

    PubMed

    Dracoulis, G D; Walker, P M; Kondev, F G

    2016-07-01

    The structure of nuclear isomeric states is reviewed in the context of their role in contemporary nuclear physics research. Emphasis is given to high-spin isomers in heavy nuclei, with [Formula: see text]. The possibility to exploit isomers to study some of the most exotic nuclei is a recurring theme. In spherical nuclei, the role of octupole collectivity is discussed in detail, while in deformed nuclei the limitations of the K quantum number are addressed. Isomer targets and isomer beams are considered, along with applications related to energy storage, astrophysics, medicine, and experimental advances. PMID:27243336

  5. Mirror nuclei constraint in nuclear mass formula

    SciTech Connect

    Wang Ning; Liang Zuoying; Liu Min; Wu, Xizhen

    2010-10-15

    The macroscopic-microscopic mass formula is further improved by considering mirror nuclei constraint. The rms deviation with respect to 2149 measured nuclear masses is reduced to 0.441 MeV. The shell corrections, the deformations of nuclei, the neutron and proton drip lines, and the shell gaps are also investigated to test the model. The rms deviation of {alpha}-decay energies of 46 superheavy nuclei is reduced to 0.263 MeV. The predicted central position of the superheavy island could lie around N=176{approx}178 and Z=116{approx}120 according to the shell corrections of nuclei.

  6. Review of metastable states in heavy nuclei

    NASA Astrophysics Data System (ADS)

    Dracoulis, G. D.; Walker, P. M.; Kondev, F. G.

    2016-07-01

    The structure of nuclear isomeric states is reviewed in the context of their role in contemporary nuclear physics research. Emphasis is given to high-spin isomers in heavy nuclei, with A≳ 150 . The possibility to exploit isomers to study some of the most exotic nuclei is a recurring theme. In spherical nuclei, the role of octupole collectivity is discussed in detail, while in deformed nuclei the limitations of the K quantum number are addressed. Isomer targets and isomer beams are considered, along with applications related to energy storage, astrophysics, medicine, and experimental advances.

  7. Mass-23 nuclei in astrophysics

    NASA Astrophysics Data System (ADS)

    Fraser, P. R.; Amos, K.; Canton, L.; Karataglidis, S.; Svenne, J. P.; van der Kniff, D.

    2015-09-01

    The formation of mass-23 nuclei by radiative capture is of great interest in astrophysics. A topical problem associated with these isobars is the so-called 22Na puzzle of ONe white dwarf novae, where the abundance of 22Na observed is not as is predicted by current stellar models, indicating there is more to learn about how the distribution of elements in the universe occurred. Another concerns unexplained variations in elements abundance on the surface of aging red giant stars. One method for theoretically studying nuclear scattering is the Multi-Channel Algebraic Scattering (MCAS) formalism. Studies to date have used a simple collective-rotor prescription to model the target states which couple to projectile nucleons. While, in general, the target states considered all belong to the ground state rotor band, for some systems it is necessary to include coupling to states outside of this band. Herein we discuss an extension of MCAS to allow coupling of different strengths between such states and the ground state band. This consideration is essential when studying the scattering of neutrons from 22Ne, a necessary step in studying the mass-23 nuclei mentioned above.

  8. The structure of light nuclei

    NASA Astrophysics Data System (ADS)

    Gao, H.

    2002-04-01

    In the last several years, tremendous advances both in experiment and theory have been made in understanding the structure of light nuclei. The experimental advances have benefited greatly from the new, high intensity CW machine (CEBAF) at Jefferson Lab and new experimental techniques utilizing polarization degrees of freedom at various laboratories. Tremendous progress has also been made in nuclear few-body theory, from a successful standard model of nuclear physics based on modern two-nucleon potentials as well as modern three-nucleon forces to the exact three-body calculation extended into the continuum by solving the corresponding Faddeev equations. In this talk, I will review recent experimental progress in understanding the structure of light nuclei focusing on the results of deuteron elastic form factors, deuteron tensor polarization, deuteron photodisintegration, and that of the 3He magnetic form factor. I will also highlight some recent results on the experimental search for the three-nucleon force, the short-range nucleon-nucleon correlation, and the nucleon structure study using a polarized 3He target as an effective neutron target. To summarize, I will provide some future outlook on this subject in the light of the upcoming BLAST program at the MIT-Bates Laboratory and the possible future 12 GeV upgrade at the Jefferson Lab.

  9. Selfconsistent calculations for hyperdeformed nuclei

    SciTech Connect

    Molique, H.; Dobaczewski, J.; Dudek, J.; Luo, W.D.

    1996-12-31

    Properties of the hyperdeformed nuclei in the A {approximately} 170 mass range are re-examined using the self-consistent Hartree-Fock method with the SOP parametrization. A comparison with the previous predictions that were based on a non-selfconsistent approach is made. The existence of the {open_quotes}hyper-deformed shell closures{close_quotes} at the proton and neutron numbers Z=70 and N=100 and their very weak dependence on the rotational frequency is suggested; the corresponding single-particle energy gaps are predicted to play a role similar to that of the Z=66 and N=86 gaps in the super-deformed nuclei of the A {approximately} 150 mass range. Selfconsistent calculations suggest also that the A {approximately} 170 hyperdeformed structures have neglegible mass asymmetry in their shapes. Very importantly for the experimental studies, both the fission barriers and the {open_quotes}inner{close_quotes} barriers (that separate the hyperdeformed structures from those with smaller deformations) are predicted to be relatively high, up to the factor of {approximately}2 higher than the corresponding ones in the {sup 152}Dy superdeformed nucleus used as a reference.

  10. Recent Direct Reaction Experimental Studies with Radioactive Tin Beams

    SciTech Connect

    Jones, K. L.; Ahn, S.; Allmond, J. M.; Ayres, A.; Bardayan, D. W.; Baugher, T.; Bazin, D.; Berryman, J. S.; Bey, A.; Bingham, C.; Cartegni, L.; Cerizza, G.; Chae, K. Y.; Cizewski, J. A.; Gade, A.; Galindo-Uribarri, A.; Garcia-Ruiz, R. F.; Grzywacz, R.; Howard, M. E.; Kozub, R. L.; Liang, J. F.; Manning, B.; Matoš, M.; McDaniel, S.; Miller, D.; Nesaraja, C. D.; O'Malley, P. D.; Padgett, S.; Padilla-Rodal, E.; Pain, S. D.; Pittman, S. T.; Radford, D. C.; Ratkiewicz, A.; Schmitt, K. T.; Shore, A.; Smith, M. S.; Stracener, D. W.; Stroberg, S. R.; Tostevin, J.; Varner, R. L.; Weisshaar, D.; Wimmer, K.; Winkler, R.

    2015-01-01

    Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z = 50 proton shell closure, as well as the neutron shell closures lying in the neutron-rich, N = 82, and neutron-deficient, N = 50, regions. Here, we present two examples of direct reactions on exotic tin isotopes. The first uses a one-neutron transfer reaction and a low-energy reaccelerated ISOL beam to study states in Sn-131 from across the N = 82 shell closure. The second example utilizes a one-neutron knockout reaction on fragmentation beams of neutron-deficient Sn-106,108Sn. In conclusion, In both cases, measurements of γ rays in coincidence with charged particles proved to be invaluable.

  11. Recent Direct Reaction Experimental Studies with Radioactive Tin Beams

    DOE PAGESBeta

    Jones, K. L.; Ahn, S.; Allmond, J. M.; Ayres, A.; Bardayan, D. W.; Baugher, T.; Bazin, D.; Berryman, J. S.; Bey, A.; Bingham, C.; et al

    2015-01-01

    Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z = 50 proton shell closure, as well as the neutron shell closures lying in the neutron-rich, Nmore » = 82, and neutron-deficient, N = 50, regions. Here, we present two examples of direct reactions on exotic tin isotopes. The first uses a one-neutron transfer reaction and a low-energy reaccelerated ISOL beam to study states in Sn-131 from across the N = 82 shell closure. The second example utilizes a one-neutron knockout reaction on fragmentation beams of neutron-deficient Sn-106,108Sn. In conclusion, In both cases, measurements of γ rays in coincidence with charged particles proved to be invaluable.« less

  12. Structure of A=6 Nuclei:

    NASA Astrophysics Data System (ADS)

    Abbas, Afsar

    It is commonly believed that (α-d) and 3He-3H) represent equivalent states of 6Li. It is shown here that this is not correct. These two are actually orthogonal to each other. It is shown here that these two with very different shapes and forms actually co-exist for the ground state of 6Li. This shape co-existence is the same as similar phenomenon in heavy nuclei. The puzzling anomaly of extremely small branching ratio for beta delayed deuteron emission in 6He is explained here. In addition the anomalously large branching ratio for beta delayed triton emission in 8He is explained. The cluster structure of the ground state and of the low-lying states of 6He, 6Li and 6Be is clarified.

  13. Single Pion production from Nuclei

    SciTech Connect

    Singh, S. K.; Athar, M. Sajjad; Ahmed, S.

    2007-12-21

    We have studied charged current one pion production induced by {nu}{sub {mu}}({nu}-bar{sub {mu}}) from some nuclei. The calculations have been done for the incoherent pion production processes from these nuclear targets in the {delta} dominance model and take into account the effect of Pauli blocking, Fermi motion and renormalization of {delta} properties in the nuclear medium. The effect of final state interactions of pions has also been taken into account. The numerical results have been compared with the recent results from the MiniBooNE experiment for the charged current 1{pi} production, and also with some of the older experiments in Freon and Freon-Propane from CERN.

  14. The Physics of Cometary Nuclei

    NASA Technical Reports Server (NTRS)

    Whipple, Fred L.

    1997-01-01

    The recent developments in cometary studies suggest rather low mean densities and weak structures for the nuclei. They appear to be accumulations of fairly discrete units loosely bound together, as deduced from the observations of Comet Shoemaker-Levy 9 during its encounter with Jupiter. The compressive strengths deduced from comet splitting by Opik and Sekanina are extremely low. These values are confirmed by theory developed here. assuming that Comet P/Holmes had a companion that collided with it in 1892. There follows a short discussion that suggests that the mean densities of comets should increase with comet dimensions. The place of origin of short-period comets may relate to these properties.

  15. Chemical composition of cometary nuclei

    NASA Technical Reports Server (NTRS)

    Delsemme, A. H.

    1982-01-01

    Observational evidence pertaining to the origin and composition of cometary material is reviewed. Arguments favoring the undifferentiated character of the icy conglomerate are summarized. Theoretical descriptions of the sublimation of a cometary nucleus and the velocity field of the expanding gas are presented and compared with observations. The nature of cometary dust and the atomic abundances of H, C, N, O, and S in the volatile fraction are examined, and data on the dust and volatile fractions are combined to derive elemental abundances. It is shown that O, N, and S in cometary nuclei appear to have essentially cosmic abundances but that both H and C are drastically depleted with respect to the cosmic abundances. The apparent depletion of C by a factor of more than three is discussed. It is suggested that the missing carbon might be hidden in the dust fraction in the form of heavy organic molecules or might have remained in either the primeval solar nebula or interstellar space.

  16. Radiative muon capture in nuclei

    SciTech Connect

    Doebeli, M.; Doser, M.; van Elmbt, L.; Schaad, M.W.; Truoel, P.; Bay, A.; Perroud, J.P.; Imazato, J.; Ishikawa, T.

    1988-04-01

    The energy spectra of photons following negative muon absorption in /sup 12/C, /sup 16/O, /sup 27/Al, /sup 40/Ca, /sup nat/Fe, /sup 165/Ho, and /sup 209/Bi have been measured with two NaI spectrometers. The branching ratios for the emission of high energy photons give information on the induced pseudoscalar coupling constant g/sub P/ in nuclear matter. The data for light nuclei are in agreement with the theoretical calculations using the nucleonic value of g/sub P/approx. =7g/sub A/ predicted by the partially conserved axial vector current hypothesis, while significantly lower values of g/sub P/ are required to fit the data of the heavier elements with presently existing theoretical predictions. Disregarding the remaining theoretical uncertainties, these results can be interpreted as a further indication of the renormalization of the nucleonic form factors inside the nucleus.

  17. Theory of active galactic nuclei

    NASA Technical Reports Server (NTRS)

    Shields, G. A.

    1986-01-01

    The involvement of accretion disks around supermassive black holes in the theory of active galactic nuclei (AGN) is discussed. The physics of thin and thick accretion disks is discussed and the partition between thermal and nonthermal energy production in supermassive disks is seen as uncertain. The thermal limit cycle may operate in supermassive disks (Shields, 1985), with accumulation of gas in the disk for periods of 10 to the 4th to 10 to the 7th years, punctuated by briefer outbursts during which the mass is rapidly transferred to smaller radii. An extended X-ray source in AGN is consistent with observations (Tennant and Mushotsky, 1983), and a large wind mass loss rate exceeding the central accretion rate means that only a fraction of the mass entering the disk will reach the central object; the rest being lost to the wind. Controversy in the relationship between the broad lines and the disk is also discussed.

  18. Clusterization and Deformation in Heavy Nuclei

    SciTech Connect

    Algora, A.; Cseh, J.; Darai, J.; Hess, P.O.; Antonenko, N.V.; Jolos, R.V.; Scheid, W.

    2005-11-21

    The deformation-dependence of clusterization in heavy nuclei is investigated. In particular, allowed and forbidden cluster-configurations are determined for the ground, superdeformed, and hyperdeformed states of some nuclei, based on a microscopic (effective SU(3)) selection rule. The stability of the different cluster configurations from the viewpoint of the binding energy and the dinuclear system model (DNS) is also investigated.

  19. Study of Nuclear Moments on Exotic Nuclei

    SciTech Connect

    Ishihara, Masayasu

    2010-04-30

    Nuclear moments have been measured for a few tens of light unstable nuclei located very far from the line of stability using beta-NMR methods and spin-polarized RI beams. The obtained values of those moments provided indispensable information to reveal/disentangle unique properties of exotic nuclei.

  20. Thalamic nuclei after human blunt head injury.

    PubMed

    Maxwell, William L; MacKinnon, Mary Anne; Smith, Douglas H; McIntosh, Tracy K; Graham, David I

    2006-05-01

    Paraffin-embedded blocks from the thalamus of 9 control patients, 9 moderately disabled, 12 severely disabled, and 10 vegetative head-injured patients assessed using the Glasgow Outcome Scale and identified from the Department of Neuropathology archive. Neurons, astrocytes, macrophages, and activated microglia were differentiated by Luxol fast blue/cresyl violet, GFAP, CD68, and CR3/43 staining and stereological techniques used to estimate cell number in a 28-microm-thick coronal section. Counts were made in subnuclei of the mediodorsal, lateral posterior, and ventral posterior nuclei, the intralaminar nuclei, and the related internal lamina. Neuronal loss occurred from mediodorsal parvocellularis, rostral center medial, central lateral and paracentral nuclei in moderately disabled patients; and from mediodorsal magnocellularis, caudal center medial, rhomboid, and parafascicular nuclei in severely disabled patients; and all of the above and the centre median nucleus in vegetative patients. Neuronal loss occurred primarily from cognitive and executive function nuclei, a lesser loss from somatosensory nuclei and the least loss from limbic motor nuclei. There was an increase in the number of reactive astrocytes, activated microglia, and macrophages with increasing severity of injury. The study provides novel quantitative evidence for differential neuronal loss, with survival after human head injury, from thalamic nuclei associated with different aspects of cortical activation. PMID:16772871

  1. Proton-Rich Nuclei in Nuclear Astrophysics

    SciTech Connect

    Rehm, K. E.

    2007-11-30

    The stable isotopes which we observe on Earth are to a large extent, produced in nature via a 'detour' through unstable nuclei. The reaction path leading through proton-rich nuclei is the so-called rapid proton capture process, where, starting from carbon, nitrogen and oxygen through successive capture or protons and alphas, followed by beta decays, nuclei up to the mass 100 region can be produced. In order to understand the reaction paths and the conditions at various astrophysical sites (e.g. Novae and X-ray bursts) cross sections, masses and half-lives of unstable nuclei have to be measured. In this contribution recent results involving proton-rich nuclei are discussed.

  2. Proton-rich nuclei in nuclear astrophysics.

    SciTech Connect

    Rehm, K. E.; Physics

    2007-01-01

    The stable isotopes which we observe on Earth are to a large extent, produced in nature via a 'detour' through unstable nuclei. The reaction path leading through proton-rich nuclei is the so-called rapid proton capture process, where, starting from carbon, nitrogen and oxygen through successive capture or protons and alphas, followed by beta decays, nuclei up to the mass 100 region can be produced. In order to understand the reaction paths and the conditions at various astrophysical sites (e.g. Novae and X-ray bursts) cross sections, masses and half-lives of unstable nuclei have to be measured. In this contribution recent results involving proton-rich nuclei are discussed.

  3. Nuclei embedded in an electron gas

    SciTech Connect

    Buervenich, Thomas J.; Mishustin, Igor N.; Greiner, Walter

    2007-09-15

    The properties of nuclei embedded in an electron gas are studied within the relativistic mean-field approach. These studies are relevant for nuclear properties in astrophysical environments such as neutron-star crusts and supernova explosions. The electron gas is treated as a constant background in the Wigner-Seitz cell approximation. We investigate the stability of nuclei with respect to {alpha} and {beta} decay. Furthermore, the influence of the electronic background on spontaneous fission of heavy and superheavy nuclei is analyzed. We find that the presence of the electrons leads to stabilizing effects for both {alpha} decay and spontaneous fission at high electron densities. Furthermore, the screening effect shifts the proton dripline to more proton-rich nuclei, and the stability line with respect to {beta}-decay is shifted to more neutron-rich nuclei. Implications for the creation and survival of very heavy nuclear systems are discussed.

  4. Spectroscopy of Neutron-rich Pu Nuclei

    SciTech Connect

    Chowdhury, P.; Hota, S.; Lakshmi, S.; Tandel, S. K.; Harrington, T.; Jackson, E.; Moran, K.; Shirwadkar, U.; Ahmad, I.; Carpenter, M. P.; Greene, J.; Hoffman, C. R.; Janssens, R. V. F.; Khoo, T. L.; Kondev, F. G.; Lauritsen, T.; Lister, C. J.; McCutchan, E. A.; Seweryniak, D.; Stefanescu, I.

    2011-10-28

    Spectroscopic studies of nuclei in the A{approx}250, Z{approx}100 region provide critical input to theoretical models that attempt to describe the structure and stability of the heaviest elements. We report here on new spectroscopic studies in the N = 150,151 nuclei {sup 244,245}Pu. (Z = 94). Excitations in these nuclei on the neutron-rich side of the valley of stability, accessed via inelastic and transfer reactions, complement fusion-evaporation studies of Z{>=}100 nuclei. States in {sup 244,245}Pu were populated using {sup 47}Ti and {sup 208}Pb beams incident on a {sup 244}Pu target, with delayed and prompt gamma rays detected by the Gammasphere array. The new results are discussed in the context of emerging systematics of one- and two-quasiparticle excitations in N{>=}150 nuclei.

  5. Complex band structure in neutron-deficient {sup 178}Hg

    SciTech Connect

    Kondev, F. G.; Carpenter, M. P.; Janssens, R. V. F.; Wiedenhoever, I.; Alcorta, M.; Bhattacharyya, P.; Brown, L. T.; Davids, C. N.; Fischer, S. M.; Khoo, T. L.

    2000-01-01

    Using the GAMMASPHERE array in conjunction with the Fragment Mass Analyzer, the level structure of the near drip-line nucleus {sup 178}Hg has been considerably expanded with the recoil-decay tagging technique. Of particular interest is a new rotational band which exhibits a complex decay towards the low spin states arising from both the prolate-deformed and the nearly spherical coexisting minima. It is proposed that this band is associated at low spin with an octupole vibration which is crossed at moderate frequency by a shape driving, two quasiproton excitation. (c) 1999 The American Physical Society.

  6. Decay studies of neutron deficient rare earth isotopes with OASIS

    SciTech Connect

    Gilat, J.; Nitschke, J.M.; Wilmarth, P.A.; Vierinen, K.; Firestone, R.B.

    1987-09-01

    We report results on the decay of /sup 124/Pr, /sup 124,125/Ce, /sup 124,125/La, /sup 134-136/Eu, /sup 134-136/Sm, /sup 134-136/Pm, /sup 144/Ho, /sup 141,142,144/Dy, /sup 140,141,142,144/Tb, /sup 140-142/Gd, and /sup 140-142/Eu, produced by /sup 92/Mo(H.I.,xpyn) reactions at the Berkeley SuperHILAC, and studied with the OASIS on-line mass separator facility. Half-lives, delayed proton branching ratios, ..gamma..-ray energies and intensities, partial decay schemes and several J/sup ..pi../ assignments are presented. Level systematics of the even mass Nd and Sm isotopes and of the nu h/sub 11/2/ - nu s/sub 1/2/ isomers for N = 77 are discussed.

  7. RADIO VARIABILITY IN SEYFERT NUCLEI

    SciTech Connect

    Mundell, C. G.; Ferruit, P.; Nagar, N.; Wilson, A. S.

    2009-09-20

    Comparison of 8.4 GHz radio images of a sample of eleven, early-type Seyfert galaxies with previous observations reveals possible variation in the nuclear radio flux density in five of them over a seven year period. Four Seyferts (NGC 2110, NGC 3081, MCG -6-30-15, and NGC 5273) show a decline in their 8.4 GHz nuclear flux density between 1992 and 1999, while one (NGC 4117) shows an increase; the flux densities of the remaining six Seyferts (Mrk 607, NGC 1386, Mrk 620, NGC 3516, NGC 4968, and NGC 7465) have remained constant over this period. New images of MCG -5-23-16 are also presented. We find no correlation between radio variability and nuclear radio luminosity or Seyfert nuclear type, although the sample is small and dominated by type 2 Seyferts. Instead, a possible correlation between the presence of nuclear radio variability and the absence of hundred parsec-scale radio emission is seen, with four out of five marginally resolved or unresolved nuclei showing a change in nuclear flux density, while five out of six extended sources show no nuclear variability despite having unresolved nuclear sources. NGC 2110 is the only source in our sample with significant extended radio structure and strong nuclear variability ({approx}38% decline in nuclear flux density over seven years). The observed nuclear flux variability indicates significant changes are likely to have occurred in the structure of the nucleus on scales smaller than the VLA beam size (i.e., within the central {approx}0.''1 (15 pc)), between the two epochs, possibly due to the appearance and fading of new components or shocks in the jet, consistent with previous detection of subparsec-scale nuclear structure in this Seyfert. Our results suggest that all Seyferts may exhibit variation in their nuclear radio flux density at 8.4 GHz, but that variability is more easily recognized in compact sources in which emission from the variable nucleus is not diluted by unresolved, constant flux density radio jet

  8. Star formation around active galactic nuclei

    NASA Technical Reports Server (NTRS)

    Keel, William C.

    1987-01-01

    Active galactic nuclei (Seyfert nuclei and their relatives) and intense star formation can both deliver substantial amounts of energy to the vicinity of a galactic nucleus. Many luminous nuclei have energetics dominated by one of these mechanisms, but detailed observations show that some have a mixture. Seeing both phenomena at once raises several interesting questions: (1) Is this a general property of some kinds of nuclei? How many AGNs have surround starbursts, and vice versa? (2) As in 1, how many undiscovered AGNs or starbursts are hidden by a more luminous instance of the other? (3) Does one cause the other, and by what means, or do both reflect common influences such as potential well shape or level of gas flow? (4) Can surrounding star formation tell us anything about the central active nuclei, such as lifetimes, kinetic energy output, or mechanical disturbance of the ISM? These are important points in the understanding of activity and star formation in galactic nuclei. Unfortunately, the observational ways of addressing them are as yet not well formulated. Some preliminary studies are reported, aimed at clarifying the issues involved in study of the relationships between stellar and nonstellar excitement in galactic nuclei.

  9. Thermal evolution of cometary nuclei

    NASA Astrophysics Data System (ADS)

    Prialnik, D.

    2014-07-01

    Thermal modeling of comet nuclei and similar objects involves the solution of conservation equations for energy and masses of the various components over time. For simplicity, the body is generally, but not necessarily, assumed to be of spherical shape. The processes included in such calculations are heat transfer, gas flow, dust drag, phase transitions, internal heating by various sources, internal structure alterations, surface sublimation. Physical properties --- such as the thermal conductivity, permeability, material strength, and porous structure --- are assumed, based on the best available estimates from laboratory experiments and space-mission results. Calculations employ various numerical procedures and require significant computational power, data analysis, and often sophisticated methods of graphical presentation. They start with a body of given size, mass, and composition, as well as a given orbit. The results yield properties and activity patterns that can be confronted with observations. Initial parameters may be adjusted until agreement is achieved. A glimpse into the internal structure of the object, which is inaccessible to direct observation, is thus obtained. The last decade, since the extensive overview of the subject was published (Modeling the structure and activity of comet nuclei, Prialnik, D.; Benkhoff, J.; Podolak, M., in Comets II, M. C. Festou, H. U. Keller, and H. A. Weaver, eds., University of Arizona Press, Tucson, p.359-387), thermal modeling has significantly advanced. This was prompted both by new properties and phenomena gleaned from observations, one example being main-belt comets, and the continual increase in computational power and performance. Progress was made on two fronts. On the computational side, multi-dimensional models have been developed, adaptive-grid and moving-boundaries techniques have been adopted, and long-term evolutionary calculations have become possible, even spanning the lifetime of the Solar System. On

  10. Fusion probability in heavy nuclei

    NASA Astrophysics Data System (ADS)

    Banerjee, Tathagata; Nath, S.; Pal, Santanu

    2015-03-01

    Background: Fusion between two massive nuclei is a very complex process and is characterized by three stages: (a) capture inside the potential barrier, (b) formation of an equilibrated compound nucleus (CN), and (c) statistical decay of the CN leading to a cold evaporation residue (ER) or fission. The second stage is the least understood of the three and is the most crucial in predicting yield of superheavy elements (SHE) formed in complete fusion reactions. Purpose: A systematic study of average fusion probability, , is undertaken to obtain a better understanding of its dependence on various reaction parameters. The study may also help to clearly demarcate onset of non-CN fission (NCNF), which causes fusion probability, PCN, to deviate from unity. Method: ER excitation functions for 52 reactions leading to CN in the mass region 170-220, which are available in the literature, have been compared with statistical model (SM) calculations. Capture cross sections have been obtained from a coupled-channels code. In the SM, shell corrections in both the level density and the fission barrier have been included. for these reactions has been extracted by comparing experimental and theoretical ER excitation functions in the energy range ˜5 %-35% above the potential barrier, where known effects of nuclear structure are insignificant. Results: has been shown to vary with entrance channel mass asymmetry, η (or charge product, ZpZt ), as well as with fissility of the CN, χCN. No parameter has been found to be adequate as a single scaling variable to determine . Approximate boundaries have been obtained from where starts deviating from unity. Conclusions: This study quite clearly reveals the limits of applicability of the SM in interpreting experimental observables from fusion reactions involving two massive nuclei. Deviation of from unity marks the beginning of the domain of dynamical models of fusion. Availability of precise ER cross

  11. Coupled-cluster computations of atomic nuclei.

    PubMed

    Hagen, G; Papenbrock, T; Hjorth-Jensen, M; Dean, D J

    2014-09-01

    In the past decade, coupled-cluster theory has seen a renaissance in nuclear physics, with computations of neutron-rich and medium-mass nuclei. The method is efficient for nuclei with product-state references, and it describes many aspects of weakly bound and unbound nuclei. This report reviews the technical and conceptual developments of this method in nuclear physics, and the results of coupled-cluster calculations for nucleonic matter, and for exotic isotopes of helium, oxygen, calcium, and some of their neighbors. PMID:25222372

  12. Critical Symmetry and Supersymmetry in Nuclei

    SciTech Connect

    Iachello, Francesco

    2006-04-26

    The role of dynamic symmetries and supersymmetries in nuclei is reviewed. The concept of critical symmetry, appropriate to describe bosonic systems (even-even nuclei) at the critical point of a phase transition, is introduced, and the symmetry, E(5), at the critical point of spherical to {gamma}-unstable shape phase transition, is discussed. The recently introduced concept of critical supersymmetry, appropriate to describe mixed systems of bosons and fermions (odd-even nuclei) at the critical point of a phase transition is presented. The case of a j=3/2 particle at the critical point of spherical to {gamma}-unstable transition, called E(5/4), is discussed.

  13. Separating Cloud Forming Nuclei from Interstitial Aerosol

    SciTech Connect

    Kulkarni, Gourihar R.

    2012-09-12

    It has become important to characterize the physicochemical properties of aerosol that have initiated the warm and ice clouds. The data is urgently needed to better represent the aerosol-cloud interaction mechanisms in the climate models. The laboratory and in-situ techniques to separate precisely the aerosol particles that act as cloud condensation nuclei (CCN) and ice nuclei (IN), termed as cloud nuclei (CN) henceforth, have become imperative in studying aerosol effects on clouds and the environment. This review summarizes these techniques, design considerations, associated artifacts and challenges, and briefly discusses the need for improved designs to expand the CN measurement database.

  14. Molecular outflows in starburst nuclei

    NASA Astrophysics Data System (ADS)

    Roy, Arpita; Nath, Biman B.; Sharma, Prateek; Shchekinov, Yuri

    2016-08-01

    Recent observations have detected molecular outflows in a few nearby starburst nuclei. We discuss the physical processes at work in such an environment in order to outline a scenario that can explain the observed parameters of the phenomenon, such as the molecular mass, speed and size of the outflows. We show that outflows triggered by OB associations, with NOB ≥ 105 (corresponding to a star formation rate (SFR)≥1 M⊙ yr-1 in the nuclear region), in a stratified disk with mid-plane density n0 ˜ 200-1000 cm-3 and scale height z0 ≥ 200(n0/102 cm-3)-3/5 pc, can form molecules in a cool dense and expanding shell. The associated molecular mass is ≥107 M⊙ at a distance of a few hundred pc, with a speed of several tens of km s-1. We show that a SFR surface density of 10 ≤ ΣSFR ≤ 50 M⊙ yr-1 kpc-2 favours the production of molecular outflows, consistent with observed values.

  15. Neurotransmitters of the suprachiasmatic nuclei

    PubMed Central

    Reghunandanan, Vallath; Reghunandanan, Rajalaxmy

    2006-01-01

    There has been extensive research in the recent past looking into the molecular basis and mechanisms of the biological clock, situated in the suprachiasmatic nuclei (SCN) of the anterior hypothalamus. Neurotransmitters are a very important component of SCN function. Thorough knowledge of neurotransmitters is not only essential for the understanding of the clock but also for the successful manipulation of the clock with experimental chemicals and therapeutical drugs. This article reviews the current knowledge about neurotransmitters in the SCN, including neurotransmitters that have been identified only recently. An attempt was made to describe the neurotransmitters and hormonal/diffusible signals of the SCN efference, which are necessary for the master clock to exert its overt function. The expression of robust circadian rhythms depends on the integrity of the biological clock and on the integration of thousands of individual cellular clocks found in the clock. Neurotransmitters are required at all levels, at the input, in the clock itself, and in its efferent output for the normal function of the clock. The relationship between neurotransmitter function and gene expression is also discussed because clock gene transcription forms the molecular basis of the clock and its working. PMID:16480518

  16. Chemical complexity in galactic nuclei

    NASA Astrophysics Data System (ADS)

    Martin-Pintado, Jesus

    2007-12-01

    In recent years our knowledge of the chemical complexity in the nuclei of galaxies has dramatically changed. Recent observations of the nucleus of the Milky Way, of the starburst galaxy NGC253 and of the ultraluminous infrared galaxy (ULIRG) Arp220 have shown large abundance of complex organic molecules believed to be formed on grains. The Galactic center appears to be the largest repository of complex organic molecule like aldehydes and alcohols in the galaxy. We also measure large abundance of methanol in starburst galaxies and in ULIRGs suggesting that complex organic molecules are also efficiently produced in the central region of galaxies with strong star formation activity. From the systematic observational studies of molecular abundance in regions dominated by different heating processes like shocks, UV radiation, X-rays and cosmic rays in the center of the Milky Way, we are opening the possibility of using chemistry as a diagnostic tool to study the highly obscured regions of galactic centers. The templates found in the nucleus of the Milky Way will be used to establish the main mechanisms driving the heating and the chemistry of the molecular clouds in galaxies with different type of activity. The role of grain chemistry in the chemical complexity observed in the center of galaxies will be also briefly discussed.

  17. Hunting η-bound nuclei

    NASA Astrophysics Data System (ADS)

    Machner, H.

    2010-09-01

    The η meson can be bound to atomic nuclei. Experimental search is discussed in the form of final state interaction for the reactions dp → 3Heη and dd → 4Heη. For the latter case tensor polarized deuterons were used in order to extract the s-wave strength. For both reactions complex scattering lengths are deduced: a3Heη = [± (10.7 ± 0.8+0.1-0.5) + i. (1.5 ± 2.6 +1.0-0.9)] fm and a4Heη = [±(3.1 ±0.5) + i. (0 ±0.5)] fm. In a two-nucleon transfer reaction under quasi-free conditions, p27 Al → 3HeX, was investigated. The system X can be the bound 25Mgotimesη at rest. When a possible decay of an intermediate N* (1535) is required, a highly significant bump shows up in the missing mass spectrum. The data give for a bound state a binding energy of 13.3 ±1.6 MeV and a width of σ = 4.4±1.3 MeV.

  18. Unbound Resonances in Light Nuclei

    NASA Astrophysics Data System (ADS)

    Havens, Elizabeth; Finck, Joseph; Gueye, Paul; Thoennessen, Michael; MoNA Collaboration

    2014-09-01

    Currently there has been no comprehensive study undertaken to compile experimental results from neutron unbound spectroscopy using invariant mass measurements, gamma resolutions, and half-lives. At Central Michigan University, Hampton University, and the NSCL, a project was initiated to catalog all unbound resonances in light nuclei (Z = 1-12). Unbound resonances were characterized by having a confirmed neutron decay branch and/or an energy level greater than the neutron binding energy listed for that isotope according to either the National Nuclear Data Center's Evaluated Nuclear Structure Files or Experimental Unevaluated Nuclear Data List and the referred journals therein. Unbound resonances will be presented for twelve elements: H, He, Li, Be, B, C, N, O, Fl, Ne, Na, and Mg. The isotopes in which unbound resonances occur will be identified, along with unbound energy levels for these isotopes. If known, each unbound resonance's gamma resolution, half-life, method of production and journal reference were also determined and a selection of these will be presented.

  19. The morphology of cometary nuclei

    NASA Astrophysics Data System (ADS)

    Keller, H. U.; Jorda, L.

    comets display residual activity or clouds of dust grains around their nuclei. Taking the residual signal into account (mostly using simple models for the brightness distribution) the size estimates of the nuclei could be improved. The (nuclear) magnitude of a comet depends on the product of its albedo and cross-section. Only in a few cases could the albedo and size of a cometary nucleus be separated by additional observation of its thermal emission at infrared wavelengths. By comparison with outer Solar System asteroids Cruikshank et al. (1985) derived a surprisingly low albedo of about 0.04. A value in clear contradiction to the perception of an icy surface but fully confirmed by the first resolved images of a cometary nucleus during the flybys of the Vega and Giotto spacecraft of comet Halley (Sagdeev et al. 1986, Keller et al. 1986). The improvements of radar techniques led to the detection of reflected signals and finally to the derivation of nuclear dimensions and rotation rates. The observations, however, are also model dependent (rotation and size are similarly interwoven as are albedo and size) and sensitive to large dust grains in the vicinity of a nucleus. As an example, Kamoun et al. (1982) determined the radius of comet Encke to 1.5 (2.3, 1.0) km using the spin axis determination of Whipple and Sekanina (1979). The superb spatial resolution of the Hubble Space Telescope (HST) is not quite sufficient to resolve a cometary nucleus. The intensity distribution of the inner coma, however, can be observed and extrapolated toward the nucleus based on models of the dust distribution. If this contribution is subtracted from the central brightness the signal of the nucleus can be derived and hence its product of albedo times cross-section (Lamy and Toth 1995, Rembor 1998, Keller and Rembor 1998; Section 4.3). It has become clear that cometary nuclei are dark, small, often irregular bodies with dimensions ranging from about a kilometre (comet Wirtanen, the target of

  20. Clusterization and quadrupole deformation in nuclei

    SciTech Connect

    Cseh, J.; Algora, A.; Antonenko, N. V.; Jolos, R. V.; Scheid, W.; Darai, J.; Hess, P. O.

    2006-04-26

    We study the interrelation of the clusterization and quadrupole deformation of atomic nuclei, by applying cluster models. Both the energetic stability and the exclusion principle is investigated. Special attention is paid to the relative orientations of deformed clusters.

  1. From Nucleons To Nuclei To Fusion Reactions

    SciTech Connect

    Quaglioni, S; Navratil, P; Roth, R; Horiuchi, W

    2012-02-15

    Nuclei are prototypes of many-body open quantum systems. Complex aggregates of protons and neutrons that interact through forces arising from quantum chromo-dynamics, nuclei exhibit both bound and unbound states, which can be strongly coupled. In this respect, one of the major challenges for computational nuclear physics, is to provide a unified description of structural and reaction properties of nuclei that is based on the fundamental underlying physics: the constituent nucleons and the realistic interactions among them. This requires a combination of innovative theoretical approaches and high-performance computing. In this contribution, we present one of such promising techniques, the ab initio no-core shell model/resonating-group method, and discuss applications to light nuclei scattering and fusion reactions that power stars and Earth-base fusion facilities.

  2. Few-Body Universality in Halo Nuclei

    NASA Astrophysics Data System (ADS)

    Hammer, H.-W.

    2016-03-01

    Few-body systems with resonant S-wave interactions show universal properties which are independent of the interaction at short distances. These properties include a geometric spectrum of three- and higher-body bound states and universal correlations between few-body observables. They can be observed on a wide range of scales from hadrons and nuclei to ultracold atoms. In this contribution, we focus on few-body universality in halo nuclei which can be considered as effective few-body systems consisting of halo nucleons and a core. This concept provides a unifying framework for halo nuclei with calculable corrections. Recent progress in this field with an emphasis on the possibility of finding Efimov states in halo nuclei is discussed.

  3. Infrared Observations of Cometary Dust and Nuclei

    NASA Technical Reports Server (NTRS)

    Lisse, Carey

    2004-01-01

    This bibliography lists citations for publications published under the grant. Subjects of the publications include cometary dust, instellar and interplanetary dust, comet nuclei and comae, Comet Hale-Bopp, infrared observations of comets, mass loss, and comet break-up.

  4. Superheavy Nuclei - Clusters of Matter and Antimatter

    SciTech Connect

    Greiner, Walter; Buervenich, Thomas J.

    2005-03-31

    The extension of the periodic system into various new areas is investigated. Experiments for the synthesis of superheavy elements and the predictions of magic numbers with modern meson field theories are reviewed. Different channels of nuclear decay are discussed including cluster radioactivity, cold fission and cold multifragmentation Furthermore, we present the vacuum for the e+-e- field of QED and show how it is modified for baryons in nuclear environment. Then we discuss the possibility of producing new types of nuclear systems by implanting an antibaryon into ordinary nuclei. The structure of nuclei containing one antiproton or antilambda is investigated within the framework of a relativistic mean-field model. Self-consistent calculations predict very enhanced binding and considerable compression in such systems as compared with normal nuclei. We present arguments that the life time of such nuclei with respect to the antibaryon annihilation might be long enough for their observation. A perspective for future research is given.

  5. True ternary fission of superheavy nuclei

    SciTech Connect

    Zagrebaev, V. I.; Karpov, A. V.; Greiner, Walter

    2010-04-15

    True ternary fission with formation of a heavy third fragment is quite possible for superheavy nuclei because of the strong shell effects leading to a three-body clusterization with the two doubly magic tinlike cores. The simplest way to discover this phenomenon in the decay of excited superheavy nuclei is a detection of two tinlike clusters with appropriate kinematics in low-energy collisions of medium-mass nuclei with actinide targets. The three-body quasi-fission process could be even more pronounced for giant nuclear systems formed in collisions of heavy actinide nuclei. In this case a three-body clusterization might be proved experimentally by the detection of two coincident leadlike fragments in low-energy U + U collisions.

  6. The Heavy Nuclei Explorer (HNX) Mission

    NASA Technical Reports Server (NTRS)

    Binns, W. R.

    2001-01-01

    The Heavy Nuclei eXplorer (HNX) mission was recently selected by NASA for a Small Explorer (SMEX) Mission Concept Study to begin in 2001. The primary scientific objectives of HNX are to measure the age of the galactic cosmic rays (GCR) since nucleosynthesis, determine the injection mechanism for the GCR accelerator (Volatility or FIP), and study the mix of nucleosynthetic processes that contribute to the source of GCRs. The experimental goal of HNX is to measure the elemental abundances of all individual stable nuclei from neon through the actinides and possibly beyond. HNX is composed of two instruments: ECCO, which measures elemental abundances of nuclei with Z(sup 3)72, and ENTICE, which measures elemental abundances of nuclei with 10(f)Z(f)82. We will discuss the mission and the science that can be addressed by HNX.

  7. Perspectives of production of superheavy nuclei

    NASA Astrophysics Data System (ADS)

    Adamian, G. G.; Antonenko, N. V.; Bezbakh, A. N.; Sargsyan, V. V.; Scheid, W.

    2016-07-01

    Possible ways of production of superheavies are discussed. Impact of nuclear structure on the production of superheavy nuclei in complete fusion reactions is discussed. The proton shell closure at Z = 120 is discussed.

  8. Where Should the Nuclei Be Located?

    ERIC Educational Resources Information Center

    Ying Liu; Yue Liu; Drew, Michael G. B.

    2005-01-01

    The approach of determining the nature of the electron wave function via orbital representations qualitatively and via numerical calculations quantitatively is demonstrated. The angular part of the wave function provides suitable representation of the positions of the nuclei.

  9. Understanding nuclei in the upper sd - shell

    SciTech Connect

    Sarkar, M. Saha; Bisoi, Abhijit; Ray, Sudatta; Kshetri, Ritesh; Sarkar, S.

    2014-08-14

    Nuclei in the upper-sd shell usually exhibit characteristics of spherical single particle excitations. In the recent years, employment of sophisticated techniques of gamma spectroscopy has led to observation of high spin states of several nuclei near A ≃ 40. In a few of them multiparticle, multihole rotational states coexist with states of single particle nature. We have studied a few nuclei in this mass region experimentally, using various campaigns of the Indian National Gamma Array setup. We have compared and combined our empirical observations with the large-scale shell model results to interpret the structure of these nuclei. Indication of population of states of large deformation has been found in our data. This gives us an opportunity to investigate the interplay of single particle and collective degrees of freedom in this mass region.

  10. Organization of projections from the raphe nuclei to the vestibular nuclei in rats

    NASA Technical Reports Server (NTRS)

    Halberstadt, A. L.; Balaban, C. D.

    2003-01-01

    Previous anatomic and electrophysiological evidence suggests that serotonin modulates processing in the vestibular nuclei. This study examined the organization of projections from serotonergic raphe nuclei to the vestibular nuclei in rats. The distribution of serotonergic axons in the vestibular nuclei was visualized immunohistochemically in rat brain slices using antisera directed against the serotonin transporter. The density of serotonin transporter-immunopositive fibers is greatest in the superior vestibular nucleus and the medial vestibular nucleus, especially along the border of the fourth ventricle; it declines in more lateral and caudal regions of the vestibular nuclear complex. After unilateral iontophoretic injections of Fluoro-Gold into the vestibular nuclei, retrogradely labeled neurons were found in the dorsal raphe nucleus (including the dorsomedial, ventromedial and lateral subdivisions) and nucleus raphe obscurus, and to a minor extent in nucleus raphe pallidus and nucleus raphe magnus. The combination of retrograde tracing with serotonin immunohistofluorescence in additional experiments revealed that the vestibular nuclei receive both serotonergic and non-serotonergic projections from raphe nuclei. Tracer injections in densely innervated regions (especially the medial and superior vestibular nuclei) were associated with the largest numbers of Fluoro-Gold-labeled cells. Differences were observed in the termination patterns of projections from the individual raphe nuclei. Thus, the dorsal raphe nucleus sends projections that terminate predominantly in the rostral and medial aspects of the vestibular nuclear complex, while nucleus raphe obscurus projects relatively uniformly throughout the vestibular nuclei. Based on the topographical organization of raphe input to the vestibular nuclei, it appears that dense projections from raphe nuclei are colocalized with terminal fields of flocculo-nodular lobe and uvula Purkinje cells. It is hypothesized that

  11. Nucleon-induced fission cross sections of heavy nuclei in the intermediate energy region

    NASA Astrophysics Data System (ADS)

    Prokofiev, Alexander V.

    Fission is the most important nuclear reaction for society at large today due to its use in energy production. However, this has raised the problem of how to treat the long-lived radioactive waste from nuclear reactors. A radical solution would be to change the composition of the waste into stable or short-lived nuclides, which could be done through nuclear transmutation. Such a concept requires accelerator-driven systems to be designed, where those for transmutation are reactor hybrids. This thesis is a contribution to the knowledge base for developing transmutation systems, specifically with respect to the computational modeling of the underlying nuclear reactions, induced by the incident and secondary particles. Intermediate energy fission cross sections are one important type of such data. Moreover, they are essential for understanding the fission process itself and related nuclear interactions. The experimental part of this work was performed at the neutron beam facility of The Svedberg Laboratory in Uppsala. Fission cross sections of 238U, 209Bi, natPb, 208Pb, 197Au, natW, and 181Ta were measured for neutrons in the range En = 30-160 MeV using thin-film breakdown counters for the fission fragment detection. A model was developed for the determination of the efficiency of such detectors. A compilation of existing data on proton-induced fission cross sections for nuclei from 165Ho to 239Pu was performed. The results, which constitute the main body of information in this field, were added to the worldwide EXFOR database. The dependences of the cross sections on incident energy and target nucleus were studied, which resulted in systematics that make it possible to give estimates for unmeasured nuclides. Nucleon-induced fission cross sections were calculated using an extended version of the cascade exciton model. A comparison with the systematics and the experimental data obtained in the present work revealed significant discrepancies. A modification of the model

  12. Cosmic Ray Nuclei (CRN) detector investigation

    NASA Technical Reports Server (NTRS)

    Meyer, Peter; Muller, Dietrich; Lheureux, Jacques; Swordy, Simon

    1991-01-01

    The Cosmic Ray Nuclei (CRN) detector was designed to measure elemental composition and energy spectra of cosmic radiation nuclei ranging from lithium to iron. CRN was flown as part of Spacelab 2 in 1985, and consisted of three basic components: a gas Cerenkov counter, a transition radiation detector, and plastic scintillators. The results of the experiment indicate that the relative abundance of elements in this range, traveling at near relativistic velocities, is similar to those reported at lower energy.

  13. Synthesis of superheavy nuclei: Obstacles and opportunities

    NASA Astrophysics Data System (ADS)

    Zagrebaev, V. I.; Karpov, A. V.; Greiner, Walter

    2015-01-01

    There are only 3 methods for the production of heavy and superheavy (SH) nuclei, namely, fusion reactions, a sequence of neutron capture and beta(-) decay and multinucleon transfer reactions. Low values of the fusion cross sections and very short half-lives of nuclei with Z<120 put obstacles in synthesis of new elements. At the same time, an important area of SH isotopes located between those produced in the cold and hot fusion reactions remains unstudied yet. This gap could be filled in fusion reactions of 48Ca with available lighter isotopes of Pu, Am, and Cm. New neutron-enriched isotopes of SH elements may be produced with the use of a 48Ca beam if a 250Cm target would be prepared. In this case we get a real chance to reach the island of stability owing to a possible beta(+) decay of 291114 and 287112 nuclei formed in this reaction with a cross section of about 0.8 pb. A macroscopic amount of the long-living SH nuclei located at the island of stability may be produced by using the pulsed nuclear reactors of the next generation only if the neutron fluence per pulse will be increased by about three orders of magnitude. Multinucleon transfer processes look quite promising for the production and study of neutron-rich heavy nuclei located in upper part of the nuclear map not reachable by other reaction mechanisms. Reactions with actinide beams and targets are of special interest for synthesis of new neutron-enriched transfermium nuclei and not-yet-known nuclei with closed neutron shell N=126 having the largest impact on the astrophysical r-process. The estimated cross sections for the production of these nuclei allows one to plan such experiments at currently available accelerators.

  14. Reaction cross sections of unstable nuclei

    SciTech Connect

    Ozawa, Akira

    2006-11-02

    Experimental studies on reaction cross sections are reviewed. The recent developments of radioactive nuclear beams have enabled us to measure reaction cross-sections for unstable nuclei. Using Glauber-model analysis, effective nuclear matter density distributions of unstable nuclei can be studied. Recent measurements in RIBLL at IMP and RIPS at RIKEN are introduced. The effective matter density distributions for 14-18C are also mentioned.

  15. New type of asymmetric fission in proton-rich nuclei.

    PubMed

    Andreyev, A N; Elseviers, J; Huyse, M; Van Duppen, P; Antalic, S; Barzakh, A; Bree, N; Cocolios, T E; Comas, V F; Diriken, J; Fedorov, D; Fedosseev, V; Franchoo, S; Heredia, J A; Ivanov, O; Köster, U; Marsh, B A; Nishio, K; Page, R D; Patronis, N; Seliverstov, M; Tsekhanovich, I; Van den Bergh, P; Van De Walle, J; Venhart, M; Vermote, S; Veselsky, M; Wagemans, C; Ichikawa, T; Iwamoto, A; Möller, P; Sierk, A J

    2010-12-17

    A very exotic process of β-delayed fission of 180Tl is studied in detail by using resonant laser ionization with subsequent mass separation at ISOLDE (CERN). In contrast to common expectations, the fission-fragment mass distribution of the post-β-decay daughter nucleus 180Hg (N/Z=1.25) is asymmetric. This asymmetry is more surprising since a mass-symmetric split of this extremely neutron-deficient nucleus would lead to two 90Zr fragments, with magic N=50 and semimagic Z=40. This is a new type of asymmetric fission, not caused by large shell effects related to fragment magic proton and neutron numbers, as observed in the actinide region. The newly measured branching ratio for β-delayed fission of 180Tl is 3.6(7) × 10(-3)%, approximately 2 orders of magnitude larger than in an earlier study. PMID:21231583

  16. Reaction theories for exotic nuclei

    SciTech Connect

    Bonaccorso, Angela

    2012-11-20

    This contribution discusses two important dynamical effects in the scattering of exotic beams. The first part deals proton breakup. The Coulomb interactions between the core and the target and the proton and the target are treated to all orders, including also the full multipole expansion of the Coulomb potential. The dynamics of proton Coulomb breakup is compared to that of an equivalent neutron of larger binding energy in order to elucidate the differences with the well understood neutron breakup mechanism. With respect to nuclear breakup it is found that a proton behaves exactly as a neutron of larger binding energy. The extra 'effective energy' is due to the combined core-target Coulomb barrier. In Coulomb breakup we distinguish the effect of the core-target Coulomb potential (called recoil effect), with respect to which the proton behaves again as a more bound neutron, from the direct proton-target Coulomb potential. The latter gives cross sections about an order of magnitude larger than the recoil term. The two effects give rise to complicated interferences in the parallel momentum distributions. They are instead easily separable in the proton angular distributions which are therefore suggested as a very useful observable for future experimental studies. The second part has to do with the dynamics of one-neutron and one-proton removal from unstable nuclei with large asymmetry {Delta}S S{sub n}-S{sub p} in the separation energies and incident energies below 80 MeV/nucleon. Strong non-sudden effects are observed in the case of deeply-bound-nucleon removal. The corresponding parallel momentum distributions exhibit an abrupt cutoff at high momentum that corresponds to an energy threshold occurring when the incident energy per particle is of comparable magnitude as the nucleon separation energy.

  17. Properties of the hypothetical spherical superheavy nuclei

    SciTech Connect

    Smolanczuk, R. |

    1997-08-01

    Theoretical results on the ground-state properties of the hypothetical spherical superheavy atomic nuclei are presented and discussed. Even-even isotopes of elements Z=104{minus}120 are considered. Certain conclusions are also drawn for odd-A and odd-odd superheavy nuclei. Results obtained earlier for even-even deformed superheavy nuclei with Z=104{minus}114 are given for completeness. Equilibrium deformation, nuclear mass, {alpha}-decay energy, {alpha}-decay half-life, dynamical fission barrier, as well as spontaneous-fission half-life are considered. {beta}-stability of superheavy nuclei is also discussed. The calculations are based on the macroscopic-microscopic model. A multidimensional deformation space describing axially symmetric nuclear shapes is used in the analysis of masses and decay properties of superheavy nuclei. We determined the boundaries of the region of superheavy nuclei which are expected to live long enough to be detected after the synthesis in a present-day experimental setup. {copyright} {ital 1997} {ital The American Physical Society}

  18. Major new sources of biological ice nuclei

    NASA Astrophysics Data System (ADS)

    Moffett, B. F.; Hill, T.; Henderson-Begg, S. K.

    2009-12-01

    Almost all research on biological ice nucleation has focussed on a limited number of bacteria. Here we characterise several major new sources of biogenic ice nuclei. These include mosses, hornworts, liverworts and cyanobacteria. Ice nucleation in the eukaryotic bryophytes appears to be ubiquitous. The temperature at which these organisms nucleate is that at which the difference in vapour pressure over ice and water is at or close to its maximum. At these temperatures (-8 to -18 degrees C) ice will grow at the expense of supercooled water. These organisms are dependent for their water on occult precipitation - fog, dew and cloudwater which by its nature is not collected in conventional rain gauges. Therefore we suggest that these organism produce ice nuclei as a water harvesting mechanism. Since the same mechanism would also drive the Bergeron-Findeisen process, and as moss is known to become airborne, these nuclei may have a role in the initiation of precipitation. The properties of these ice nuclei are very different from the well characterised bacterial nuclei. We will also present DNA sequence data showing that, although related, the proteins responsible are only very distantly related to the classical bacterial ice nuclei.

  19. 76 FR 63702 - In the Matter of the Designation of Conspiracy of Fire Nuclei, aka Conspiracy of the Nuclei of...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-10-13

    ... Matter of the Designation of Conspiracy of Fire Nuclei, aka Conspiracy of the Nuclei of Fire, aka Conspiracy of Cells of Fire, aka Synomosia of Pyrinon Tis Fotias, aka Thessaloniki-Athens Fire Nuclei... January 23, 2003, I hereby determine that the organization known as Conspiracy of Fire Nuclei, also...

  20. Harvard--MIT research program in short-lived radiopharmaceuticals

    SciTech Connect

    Not Available

    1991-03-01

    This report describes progress on five projects. The first project showed a 1000 fold concentration of the cationic complex {sup 99m}Tc (MIBI) in heart cell mitochondria vs heart cell cytoplasm, as determined by high resolution electron probe microanalysis. Additional technetium-99m based complexes are being developed and tested. The second project involves evaluating technetium acetylacteonates as potential indicators of cerebral blood flow. An intermediate in the synthesis of a technetium porphyrin complex has been synthesized; an oxotechnetium(V)-2,4-pentanedione complex has been prepared and is currently being characterized. The third project involves using radio labelled antibodies for diagnosis and treatment of cancer. An early discovery was that chloramine-T based iodination protocols resulted in a reversal of the charge on mouse lgGs. Immunoperoxidase-labelled monoclonal antibody MOv 18 was shown to bind specifically to the most frequent ovarian aderon carcinomas, and not to healthy tissue, making this antibody a good candidate for immunotherapy or immunodetection. Work on a specific immunotherapy protocol suffered a setback when one reagent, a {sup 125}I-biotin complex, proved to be unstable in vivo. The fourth project involves labelling antibodies with positron emitting radionuclides. Radiofluorination was accomplished through reductive alkylation of {sup 18}F-aldehyde, or pentafluorophenyl esters. Radioiodination was accomplished using alkyl-tin derivation exchange. The fifth project examined antibody modification for use in radioimmune imaging. Technetium-99m-labelled lgG was shown to be biologically equivalent to Indium-III-labelled lgG for imaging focal sites of inflamation. Also, Indium III labelling of small bioactive peptides was examined as a means of imaging important physiological processes. 44 refs., 2 figs.

  1. Short-lived Rn-222 daughters in cryogenic liquids

    NASA Astrophysics Data System (ADS)

    Pelczar, Krzysztof; Frodyma, Nikodem; Wójcik, Marcin

    2013-08-01

    In this paper a detection method of α emitters from 222Rn decay chain, present in cryogenic liquids, using bare Si-PIN diodes immersed in the liquids is presented. Properties of ionized 222Rn daughters deduced from conducted measurements are outlined. Life-time of positive ions was found to be of the order of 10 s, and nonzero content of electronegative ions was observed.

  2. Production of a short-lived filament by a surge

    NASA Technical Reports Server (NTRS)

    Zirin, H.

    1976-01-01

    A large surge was observed on September 17, 1971 part of which, after travelling 200,000 km across the surface, returned to the surface to form a filament. The filament lasted about 30 minutes, then rose up and returned to the source of the surge. This was interpreted as the filling of a semi-stable magnetic trap. Analysis of the microwave radio burst showed it to have been produced by a source optically thick at 8,800 MHz, with area 4 (arc min)squared and T approximately 275,000 deg, N squared sub eV approximately 7 x 10 to the 48th power. The soft x-ray burst showed a component at 12 x 1,00.000 deg with N squared sub eV approximately 3 x 10 to the 48th power.

  3. Short-lived radionuclides in nuclear medicine - II

    SciTech Connect

    Budinger, T.F.; Peng, C.T.

    1985-11-01

    Positron emission tomography (PET) has been applied effectively in the diagnosis of Alzheimer's disease, the prognosis of stroke, and the evaluation of the efficacy of tumor therapy. In addition, PET has been applied to studies of the neuroreceptor distribution in the human brain, to studies of epilepsy and congenital disorders of the brain, and to the study of flow and metabolism of the human heart muscle. Of the many current investigations of PET, the three discussed here are now of clinical importance for patient care.

  4. Tropospheric Ozone as a Short-lived Chemical Climate Forcer

    NASA Technical Reports Server (NTRS)

    Pickering, Kenneth E.

    2012-01-01

    Tropospheric ozone is the third most important greenhouse gas according to the most recent IPCC assessment. However, tropospheric ozone is highly variable in both space and time. Ozone that is located in the vicinity of the tropopause has the greatest effect on climate forcing. Nitrogen oxides (NOx) are the most important precursors for ozone In most of the troposphere. Therefore, pollution that is lofted upward in thunderstorm updrafts or NOx produced by lightning leads to efficient ozone production in the upper troposphere, where ozone is most important climatically. Global and regional model estimates of the impact of North American pollution and lightning on ozone radiative forcing will be presented. It will be shown that in the Northern Hemisphere summer, the lightning effect on ozone radiative forcing can dominate over that of pollution, and that the radiative forcing signal from North America extends well into Europe and North Africa. An algorithm for predicting lightning flash rates and estimating lightning NOx emissions is being incorporated into the NASA GEOS-5 Chemistry and Climate Model. Changes in flash rates and emissions over an ENSO cycle and in future climates will be assessed, along with the resulting changes in upper tropospheric ozone. Other research on the production of NOx per lightning flash and its distribution in the vertical based on cloud-resolving modeling and satellite observations will be presented. Distributions of NO2 and O3 over the Middle East from the OMI instrument on NASA's Aura satellite will also be shown.

  5. Short-lived isomers in 192Po and 194Po

    NASA Astrophysics Data System (ADS)

    Andel, B.; Andreyev, A. N.; Antalic, S.; Heßberger, F. P.; Ackermann, D.; Hofmann, S.; Huyse, M.; Kalaninová, Z.; Kindler, B.; Kojouharov, I.; Kuusiniemi, P.; Lommel, B.; Nishio, K.; Page, R. D.; Sulignano, B.; Van Duppen, P.

    2016-06-01

    Isomeric states in 194Po and 192Po were studied at the velocity filter SHIP. The isotopes were produced in the fusion-evaporation reactions 141Pr(56Fe, p 2 n )194Po and 144Sm(51V, p 2 n )192Po . Several new γ -ray transitions were attributed to the isomers and γ -γ coincidences for both isomers were studied for the first time. The 459-keV transition earlier, tentatively proposed as de-exciting the isomeric level in 194Po, was replaced by a new 248-keV transition, and the spin of this isomer was reassigned from (11-) to (10-). The de-excitation of the (11-) isomeric level in 192Po by the 154-keV transition was confirmed and a parallel de-excitation by a 733-keV (E 3 ) transition to (8+) level of the ground-state band was suggested. Moreover, side feeding to the (4+) level of the ground-state band was proposed. The paper also discusses strengths of transitions de-exciting 11- isomers in neighboring Po and Pb isotopes.

  6. Malaria Vaccine Protection Short-Lived in Young Children

    MedlinePlus

    ... a situation where unvaccinated children have more natural immunity than vaccinated children, and therefore get less malaria," ... may allow a person to develop some natural immunity to the parasite, Plowe suggested. "You're basically ...

  7. Malaria Vaccine Protection Short-Lived in Young Children

    MedlinePlus

    ... was published June 30 in the New England Journal of Medicine . SOURCES: Philip Bejon, Ph.D., director, Kenya Medical Research Institute-Wellcome Trust Program, Kilifi, Kenya; Christopher Plowe, ...

  8. Harvard-MIT research program in short-lived radiopharmaceuticals

    SciTech Connect

    Adelstein, S.J.

    1991-01-01

    This report presents research on radiopharmaceuticals. The following topics are discussed: antibody labeling with positron-emitting radionuclides; antibody modification for radioimmune imaging; labeling antibodies; evaluation of technetium acetlyacetonates as potential cerebral blood flow agents; and studies in technetium chemistry. (CBS)

  9. Zirovski Vrh: A short-lived uranium producer

    SciTech Connect

    Pool, T.C.

    1993-09-01

    The Zirovski Vrh uranium deposit, located in Slovenia, formerly a province of Yugoslavia, was discovered and explored in an era of increasing interest in the commercial possibilities of nuclear power. Its development and exploitation were planned and designed specifically to provide fuel for the country's only nuclear reactor; Krsko, a 632-MWe pressurized water reactor, during a period when uranium seemed in short supply. It was designed as a model of compact efficiency, state of the art technology, and environmental sensitivity. By the time it achieved production, however, uranium prices were rapidly declining and production facilities were under increasing pressure from environmental activists. Even its status as a state-supported enterprise failed to insulate it from the economic pressures of the marketplace. Was the mine a victim of bad timing or poor fundamentals In short, the Zirovski Vrh mine was founded upon a low-grade, conventional underground mining situation with limited flexibility. Even with prices at $40 per pound, the mine was a marginal producer.

  10. On Al-26 and other short-lived interstellar radioactivity

    NASA Technical Reports Server (NTRS)

    Clayton, Donald D.; Hartmann, Dieter H.; Leising, Mark D.

    1993-01-01

    Several authors have shown that massive stars exploding at a rate of about three per century can account for a large portion, if not all, of the observed interstellar Al-26. In a separate argument using models of Galactic chemical evolution, Clayton (1984) showed that the Al-26/Al-27 production ratio was not large enough to maintain enough Al-26 in the Galactic disk gas of about 10 exp 10 solar masses having solar composition. We present a resolution of those conflicting arguments. A past history of Galactic infall growing the Galactic disk so dilutes the stable Al-27 concentration that the two approaches can be brought into near agreement. If massive stars dominate the production of Al-26, we suggest that the apparent shortfall of their Al-26/Al-27 yield ratio is to be interpreted as evidence for significant growth of the Galactic disk. We also discuss the implications of these arguments for other extinct radioactivities in meteorites, using I-129 and Sm-146 as examples.

  11. Short-lived Rn-222 daughters in cryogenic liquids

    SciTech Connect

    Pelczar, Krzysztof; Frodyma, Nikodem; Wójcik, Marcin

    2013-08-08

    In this paper a detection method of α emitters from {sup 222}Rn decay chain, present in cryogenic liquids, using bare Si-PIN diodes immersed in the liquids is presented. Properties of ionized {sup 222}Rn daughters deduced from conducted measurements are outlined. Life-time of positive ions was found to be of the order of 10 s, and nonzero content of electronegative ions was observed.

  12. 8Be and 9B nuclei in dissociation of relativistic 10B and 11C nuclei

    NASA Astrophysics Data System (ADS)

    Artemenkov, D. A.; Bradnova, V.; Firu, E.; Kornegrutsa, N. K.; Haiduc, M.; Mamatkulov, K. Z.; Kattabekov, R. R.; Neagu, A.; Rukoyatkin, P. A.; Rusakova, V. V.; Stanoeva, R.; Zaitsev, A. A.; Zarubin, P. I.; Zarubina, I. G.

    2016-02-01

    Progress in the study of nuclear clustering in the relativistic 10B and 11C nuclei dissociation in nuclear track emulsion is presented. The contribution of the unbound 8Be and 9B nuclei to their structure is determined on the basis of measurements of the emission angles of relativistic He and H fragments.

  13. 8Be and 9B nuclei in dissociation of relativistic 10C and 11C nuclei

    NASA Astrophysics Data System (ADS)

    Artemenkov, D. A.; Bradnova, V.; Firu, E.; Kornegrutsa, N. K.; Haiduc, M.; Mamatkulov, K. Z.; Kattabekov, R. R.; Neagu, A.; Rukoyatkin, P. A.; Rusakova, V. V.; Stanoeva, R.; Zaitsev, A. A.; Zarubin, P. I.; Zarubina, I. G.

    2016-05-01

    Progress in the study of nuclear clustering in the relativistic 10C and 11C nuclei dissociation in nuclear track emulsion is presented. The contribution of the unbound 8Be and 9B nuclei to their structure is determined on the basis of measurements of the emission angles of relativistic He and H fragments.

  14. Transition (LINER/HII) nuclei as evolved Composite (Seyfert 2/Starburst) nuclei

    NASA Astrophysics Data System (ADS)

    Storchi-Bergmann, Thaisa; Brandt, C. H.; Cid Fernandes, R.; Schmitt, H. R.; González Delgado, R.

    2004-11-01

    We compare the circumnuclear stellar population and environmental properies of Seyfert and Composite (Seyfert + Starburst) nuclei with those of LINERs and LINER/HII transition galaxies (TOs), and discuss evidence for evolution from Seyfert/Composite to LINER/TO nuclei.

  15. Compact Nuclei in Galaxies at Moderate Redshift

    NASA Astrophysics Data System (ADS)

    Sarajedini, Vicki Lynn

    The purpose of this study is to understand the space density and properties of active galaxies to z ≃ 0.8. We have investigated the frequency and nature of unresolved nuclei in galaxies at moderate redshift as indicators of nuclear activity such as Active Galactic Nuclei (AGN) or starbursts. Candidates are selected by fitting imaged galaxies with multi-component models using maximum likelihood estimate techniques to determine the best model fit. We select those galaxies requiring an unresolved, point source component in the galaxy nucleus, in addition to a disk and/or bulge component, to adequately model the galaxy light. We have searched 70 WFPC2 images primarily from the Medium Deep Survey for galaxies containing compact nuclei. In our survey of 1033 galaxies, the fraction containing an unresolved nuclear component ≥3% of the total galaxy light is 16±3% corrected for incompleteness and 9±1% for nuclei ≥5% of the galaxy light. Most of the nuclei are ~<20% of the total galaxy light. The majority of the host galaxies are spirals with little or no bulge component. The V-I colors of the nuclei are compared with synthetic colors for Seyferts and starburst nuclei to help differentiate between AGNs and starbursts in our sample. Spectroscopic redshifts have been obtained for 35 of our AGN/starburst candidates and photometric redshifts are estimated to an accuracy of σz≃0.1 for the remaining sample. We present the upper limit luminosity function (LF) for low-luminosity AGN (LLAGN) in two redshift bins to z = 0.8. We detect mild number density evolution of the form φ∝ (1+z)1.9 for nuclei at -18 ~

  16. Stability and production of superheavy nuclei

    SciTech Connect

    Moeller, P. |; Nix, J.R.

    1997-12-31

    Beyond uranium heavy elements rapidly become increasingly unstable with respect to spontaneous fission as the proton number Z increases, because of the disruptive effect of the long-range Coulomb force. However, in the region just beyond Z = 100 magic proton and neutron numbers and the associated shell structure enhances nuclear stability sufficient to allow observation of additional nuclei. Some thirty years ago it was speculated that an island of spherical, relatively stable superheavy nuclei would exist near the next doubly magic proton-neutron combination beyond {sup 208}Pb, that is, at proton number Z = 114 and neutron number N = 184. Theory and experiment now show that there also exists a rock of stability in the vicinity of Z = 110 and N = 162 between the actinide region, which previously was the end of the peninsula of known elements, and the predicted island of spherical superheavy nuclei slightly southwest of the magic numbers Z = 114 and N = 184. The authors review here the stability properties of the heavy region of nuclei. Just as the decay properties of nuclei in the heavy region depend strongly on shell structure, this structure also dramatically affects the fusion entrance channel. The six most recently discovered new elements were all formed in cold-fusion reactions. They discuss here the effect of the doubly magic structure of the target in cold-fusion reactions on the fusion barrier and on dissipation.

  17. Shape-based nuclei area of digitized pap smear images

    NASA Astrophysics Data System (ADS)

    Muhimmah, Izzati; Kurniawan, Rahadian

    2012-04-01

    Nuclei of the epithelial of Pap smear cells are important risk indicator of cervical cancers. Pathologist uses the changing of the area of the nuclei to determine whether cells are normal or abnormal. It means that having correct measurement of the area of nuclei is important on the pap smears assessment. Our paper present a novel approach to analyze the shape of nuclei in pap smear images and measuring the area of nuclei. We conducted a study to measure the area of nuclei automatically by calculating the number of pixels contained in each of the segmented nuclei. For comparison, we performed measurements of nuclei area using the ellipse area approximation. The result of the t-test confirmed that there were similarity between elliptical area approximation and automatic segmented nuclei-area at 0.5% level of significance.

  18. Quantum Monte Carlo calculations of light nuclei.

    SciTech Connect

    Pieper, S. C.; Physics

    2008-01-01

    Variational Monte Carlo and Green's function Monte Carlo are powerful tools for cal- culations of properties of light nuclei using realistic two-nucleon (NN) and three-nucleon (NNN) potentials. Recently the GFMC method has been extended to multiple states with the same quantum numbers. The combination of the Argonne v18 two-nucleon and Illinois-2 three-nucleon potentials gives a good prediction of many energies of nuclei up to 12 C. A number of other recent results are presented: comparison of binding energies with those obtained by the no-core shell model; the incompatibility of modern nuclear Hamiltonians with a bound tetra-neutron; difficulties in computing RMS radii of very weakly bound nuclei, such as 6He; center-of-mass effects on spectroscopic factors; and the possible use of an artificial external well in calculations of neutron-rich isotopes.

  19. Quantum Monte Carlo calculations of light nuclei

    SciTech Connect

    Pieper, S.C.

    1998-12-01

    Quantum Monte Carlo calculations using realistic two- and three-nucleon interactions are presented for nuclei with up to eight nucleons. We have computed the ground and a few excited states of all such nuclei with Greens function Monte Carlo (GFMC) and all of the experimentally known excited states using variational Monte Carlo (VMC). The GFMC calculations show that for a given Hamiltonian, the VMC calculations of excitation spectra are reliable, but the VMC ground-state energies are significantly above the exact values. We find that the Hamiltonian we are using (which was developed based on {sup 3}H,{sup 4}He, and nuclear matter calculations) underpredicts the binding energy of p-shell nuclei. However our results for excitation spectra are very good and one can see both shell-model and collective spectra resulting from fundamental many-nucleon calculations. Possible improvements in the three-nucleon potential are also be discussed. {copyright} {ital 1998 American Institute of Physics.}

  20. Quantum Monte Carlo calculations of light nuclei

    SciTech Connect

    Pieper, Steven C.

    1998-12-21

    Quantum Monte Carlo calculations using realistic two- and three-nucleon interactions are presented for nuclei with up to eight nucleons. We have computed the ground and a few excited states of all such nuclei with Greens function Monte Carlo (GFMC) and all of the experimentally known excited states using variational Monte Carlo (VMC). The GFMC calculations show that for a given Hamiltonian, the VMC calculations of excitation spectra are reliable, but the VMC ground-state energies are significantly above the exact values. We find that the Hamiltonian we are using (which was developed based on {sup 3}H,{sup 4}He, and nuclear matter calculations) underpredicts the binding energy of p-shell nuclei. However our results for excitation spectra are very good and one can see both shell-model and collective spectra resulting from fundamental many-nucleon calculations. Possible improvements in the three-nucleon potential are also be discussed.