Spin-current emission governed by nonlinear spin dynamics
Tashiro, Takaharu; Matsuura, Saki; Nomura, Akiyo; Watanabe, Shun; Kang, Keehoon; Sirringhaus, Henning; Ando, Kazuya
2015-01-01
Coupling between conduction electrons and localized magnetization is responsible for a variety of phenomena in spintronic devices. This coupling enables to generate spin currents from dynamical magnetization. Due to the nonlinearity of magnetization dynamics, the spin-current emission through the dynamical spin-exchange coupling offers a route for nonlinear generation of spin currents. Here, we demonstrate spin-current emission governed by nonlinear magnetization dynamics in a metal/magnetic insulator bilayer. The spin-current emission from the magnetic insulator is probed by the inverse spin Hall effect, which demonstrates nontrivial temperature and excitation power dependences of the voltage generation. The experimental results reveal that nonlinear magnetization dynamics and enhanced spin-current emission due to magnon scatterings are triggered by decreasing temperature. This result illustrates the crucial role of the nonlinear magnon interactions in the spin-current emission driven by dynamical magnetization, or nonequilibrium magnons, from magnetic insulators. PMID:26472712
Spin-current emission governed by nonlinear spin dynamics.
Tashiro, Takaharu; Matsuura, Saki; Nomura, Akiyo; Watanabe, Shun; Kang, Keehoon; Sirringhaus, Henning; Ando, Kazuya
2015-01-01
Coupling between conduction electrons and localized magnetization is responsible for a variety of phenomena in spintronic devices. This coupling enables to generate spin currents from dynamical magnetization. Due to the nonlinearity of magnetization dynamics, the spin-current emission through the dynamical spin-exchange coupling offers a route for nonlinear generation of spin currents. Here, we demonstrate spin-current emission governed by nonlinear magnetization dynamics in a metal/magnetic insulator bilayer. The spin-current emission from the magnetic insulator is probed by the inverse spin Hall effect, which demonstrates nontrivial temperature and excitation power dependences of the voltage generation. The experimental results reveal that nonlinear magnetization dynamics and enhanced spin-current emission due to magnon scatterings are triggered by decreasing temperature. This result illustrates the crucial role of the nonlinear magnon interactions in the spin-current emission driven by dynamical magnetization, or nonequilibrium magnons, from magnetic insulators. PMID:26472712
Multiferroics with spiral spin orders.
Tokura, Yoshinori; Seki, Shinichiro
2010-04-12
Cross correlation between magnetism and electricity in a solid can host magnetoelectric effects, such as magnetic (electric) induction of polarization (magnetization). A key to attain the gigantic magnetoelectric response is to find the efficient magnetism-electricity coupling mechanisms. Among those, recently the emergence of spontaneous (ferroelectric) polarization in the insulating helimagnet or spiral-spin structure was unraveled, as mediated by the spin-exchange and spin-orbit interactions. The sign of the polarization depends on the helicity (spin rotation sense), while the polarization direction itself depends on further details of the mechanism and the underlying lattice symmetry. Here, we describe some prototypical examples of the spiral-spin multiferroics, which enable some unconventional magnetoelectric control such as the magnetic-field-induced change of the polarization direction and magnitude as well as the electric-field-induced change of the spin helicity and magnetic domain. PMID:20496385
Order From disorder in Frustrated Spin Systems
NASA Astrophysics Data System (ADS)
Coleman, Piers
This talk will review the phemomenon of ''Order from disorder'': the mechanism by which fluctuations remove a degeneracy within a frustrated spin system. An important consequence of order-from-disorder, is the ability of frustrated Heisenberg spin systems to overcome the Mermin-Wagner theorem, developing new forms of discrete order, even when the spins themselves remain disordered with a finite correlation length. The most well-known example, is the two-dimensional frustrated J1 -J2 Heisenberg model, which undergoes a finite temperature Ising phase transition into a stripy or ''nematic'' state, even though the spins do not order until absolute zero. Nematic ordering of this kind is believed to occur in the iron-based superconductors, such as BaFe2 As2 . More recently, it has been possible to theoretically study the triangular-honeycomb versions of the J1 -J2 model, called a windmill model, in which order-from disorder drives the development of six-state clock order. Remarkably, in this case, order-from-disorder leads to an intermediate power-law spin phase, despite the underlying Heisenerg spins. This research was supported by DOE Basic Energy Sciences Grant DE-FG02-99ER45790.
Quadrupolar Spin Orders in FeSe
NASA Astrophysics Data System (ADS)
Wang, Zhentao; Nevidomskyy, Andriy
Motivated by the absence of long-range magnetic order and the strong spin fluctuations observed in the Fe-based superconductor FeSe, we study spin-1 model on a square lattice up to next-nearest neighbor Heisenberg and biquadratic spin exchanges. The zero-temperature variational phase diagram gives the conventional antiferromagnetic order and also more exotic quadrupolar spin phases. These quadrupolar phases do not host long-range magnetic order and preserve time-reversal symmetry, but break the spin SU(2) symmetry. In particular, we observe a robust ferroquadrupolar order (FQ) in immediate proximity to the columnar AFM phase. We envision that FeSe may be positioned within the FQ phase close to the phase boundary. Using the flavor-wave technique, we calculate the structure factor inside the FQ phase and find a Goldstone mode emerging from Q = (0 , 0) , which however bears zero spectral weight at ω = 0 due to time reversal symmetry. At the same time, we observe strong spin fluctuations near (π , 0) / (0 , π) , which agrees with the recent neutron scattering experiments. Further, we calculate the higher order interactions between the (π , 0) and (0 , π) spin fluctuations inside the FQ phase, which may shed light on the C4 symmetry breaking in the nematic phase of FeSe.
Helical Spin Order from Topological Dirac and Weyl Semimetals
NASA Astrophysics Data System (ADS)
Sun, Xiao-Qi; Zhang, Shou-Cheng; Wang, Zhong
2015-08-01
We study dynamical mass generation and the resultant helical spin orders in topological Dirac and Weyl semimetals, including the edge states of quantum spin Hall insulators, the surface states of weak topological insulators, and the bulk materials of Weyl semimetals. In particular, the helical spin textures of Weyl semimetals manifest the spin-momentum locking of Weyl fermions in a visible manner. The spin-wave fluctuations of the helical order carry electric charge density; therefore, the spin textures can be electrically controlled in a simple and predictable manner.
48 CFR 51.103 - Ordering from Government supply sources.
Code of Federal Regulations, 2010 CFR
2010-10-01
... 48 Federal Acquisition Regulations System 1 2010-10-01 2010-10-01 false Ordering from Government supply sources. 51.103 Section 51.103 Federal Acquisition Regulations System FEDERAL ACQUISITION REGULATION CONTRACT MANAGEMENT USE OF GOVERNMENT SOURCES BY CONTRACTORS Contractor Use of Government Supply Sources 51.103 Ordering from Government...
High Spin-Chern Insulators with Magnetic Order
Ezawa, Motohiko
2013-01-01
As a topological insulator, the quantum Hall (QH) effect is indexed by the Chern and spin-Chern numbers and . We have only in conventional QH systems. We investigate QH effects in generic monolayer honeycomb systems. We search for spin-resolved characteristic patterns by exploring Hofstadter's butterfly diagrams in the lattice theory and fan diagrams in the low-energy Dirac theory. It is shown that the spin-Chern number can takes an arbitrary high value for certain QH systems. This is a new type of topological insulators, which we may call high spin-Chern insulators. Samples may be provided by graphene on the SiC substrate with ferromagnetic order, transition-metal dichalcogenides with ferromagnetic order, transition-metal oxide with antiferromagnetic order and silicene with ferromagnetic order. Actually high spin-Chern insulators are ubiquitous in any systems with magnetic order. Nevertheless, the honeycomb system would provide us with unique materials for practical materialization. PMID:24310394
High Spin-Chern Insulators with Magnetic Order
NASA Astrophysics Data System (ADS)
Ezawa, Motohiko
2013-12-01
As a topological insulator, the quantum Hall (QH) effect is indexed by the Chern and spin-Chern numbers and . We have only in conventional QH systems. We investigate QH effects in generic monolayer honeycomb systems. We search for spin-resolved characteristic patterns by exploring Hofstadter's butterfly diagrams in the lattice theory and fan diagrams in the low-energy Dirac theory. It is shown that the spin-Chern number can takes an arbitrary high value for certain QH systems. This is a new type of topological insulators, which we may call high spin-Chern insulators. Samples may be provided by graphene on the SiC substrate with ferromagnetic order, transition-metal dichalcogenides with ferromagnetic order, transition-metal oxide with antiferromagnetic order and silicene with ferromagnetic order. Actually high spin-Chern insulators are ubiquitous in any systems with magnetic order. Nevertheless, the honeycomb system would provide us with unique materials for practical materialization.
Hole dynamics in spin and orbital ordered vanadium perovskites
NASA Astrophysics Data System (ADS)
Ishihara, Sumio
2005-03-01
We present a theory of the doped perovskite vanadates with spin and orbital orders [1]. Two kinds of spin-orbital orders are found in the ground state: the G-type (three-dimensional (3D) staggered) spin order (SO) with the C-type (rod type) orbital order (OO) (the alternative dxy^1dyz^1/dxy^1dzx^1 configuration) termed (SG/OC) in YVO3, and the C-type SO with the G-type OO termed (SC/OG) in LaVO3. Mobile holes are strongly renormalized by spin excitations (magnons) in the spin G-type and orbital C-type (SG/OC) order, and orbital excitations (orbitons) in the spin C-type and orbital G-type (SC/OG) one. It is found that hole dynamics in a staggered t2g orbital array is distinct from that in a antiferromagnetic order as well as the eg orbital one. The anomalously fragile character of the (SG/OC) order observed in Y1-xCaxVO3 is attributed to the orbiton softening induced by a reduction of the spin order parameter. [1] S. Ishihara, cond-mat/0408395.
Nature of ordering in Potts spin glasses
NASA Astrophysics Data System (ADS)
Banavar, Jayanth R.; Cieplak, Marek
1989-09-01
The zero-temperature scaling approach is applied to the three-state Potts spin glass. Our results suggest that the +/-J model has a lower critical dimensionality greater than 3, whereas for the Gaussian model this dimensionality is slightly less than 3. The T=0 scaling exponents are estimated in D=2 and 3. The results are based mostly on exact transfer-matrix calculations and on a Monte Carlo quenching procedure.
Chen, Xiang-Bai; Hien, Nguyen Thi Minh; Han, Kiok; Nam, Ji-Yeon; Huyen, Nguyen Thi; Shin, Seong-Il; Wang, Xueyun; Cheong, S. W.; Lee, D.; Noh, T. W.; Sung, N. H.; Cho, B. K.; Yang, In-Sang
2015-01-01
Spin-wave (magnon) scattering, when clearly observed by Raman spectroscopy, can be simple and powerful for studying magnetic phase transitions. In this paper, we present how to observe magnon scattering clearly by Raman spectroscopy, then apply the Raman method to study spin-ordering and spin-reorientation transitions of hexagonal manganite single crystal and thin films and compare directly with the results of magnetization measurements. Our results show that by choosing strong resonance condition and appropriate polarization configuration, magnon scattering can be clearly observed, and the temperature dependence of magnon scattering can be simple and powerful quantity for investigating spin-ordering as well as spin-reorientation transitions. Especially, the Raman method would be very helpful for investigating the weak spin-reorientation transitions by selectively probing the magnons in the Mn3+ sublattices, while leaving out the strong effects of paramagnetic moments of the rare earth ions. PMID:26300075
Chen, Xiang-Bai; Hien, Nguyen Thi Minh; Han, Kiok; Nam, Ji-Yeon; Huyen, Nguyen Thi; Shin, Seong-Il; Wang, Xueyun; Cheong, S W; Lee, D; Noh, T W; Sung, N H; Cho, B K; Yang, In-Sang
2015-01-01
Spin-wave (magnon) scattering, when clearly observed by Raman spectroscopy, can be simple and powerful for studying magnetic phase transitions. In this paper, we present how to observe magnon scattering clearly by Raman spectroscopy, then apply the Raman method to study spin-ordering and spin-reorientation transitions of hexagonal manganite single crystal and thin films and compare directly with the results of magnetization measurements. Our results show that by choosing strong resonance condition and appropriate polarization configuration, magnon scattering can be clearly observed, and the temperature dependence of magnon scattering can be simple and powerful quantity for investigating spin-ordering as well as spin-reorientation transitions. Especially, the Raman method would be very helpful for investigating the weak spin-reorientation transitions by selectively probing the magnons in the Mn(3+) sublattices, while leaving out the strong effects of paramagnetic moments of the rare earth ions. PMID:26300075
Charge dynamics and spin order in doped Hubbard models
Kampf, A.P.; Brenig, W.
1994-04-01
Hole motion in an antiferromagnetic (AF) environment is accompanied by the emission of spin wave excitations. Spin-wave shakeoffs are responsible for incoherent contributions to the dynamics of propagating holes. Using a spin-density-wave polaron scheme the authors calculate the optical conductivity {sigma}({omega}) and show that the incoherent part of the hole spectrum contributes to the low-frequency part of {sigma}({omega}). Separately, the authors discuss the possible formation of spiral spin patterns upon doping of the half-filled one-band Hubbard model. In particular, the authors consider the influence of band structure effects arising from nearest- and next-nearest-neighbor hopping processes on a square lattice. Differences in the ground state spin patterns for hole and electron doping are obtained offering a possible explanation for the persistence of AF order in low electron-doped cuprate superconductors.
Next-to-leading order gravitational spin(1)-spin(2) dynamics in Hamiltonian form
Steinhoff, Jan; Hergt, Steven; Schaefer, Gerhard
2008-04-15
Based on recent developments by the authors a next-to-leading order spin(1)-spin(2) Hamiltonian is derived for the first time. The result is obtained within the canonical formalism of Arnowitt, Deser, and Misner (ADM) utilizing their generalized isotropic coordinates. A comparison with other methods is given.
Field-induced ordering in dipolar spin ice
NASA Astrophysics Data System (ADS)
Kao, Wen-Han; Holdsworth, Peter C. W.; Kao, Ying-Jer
2016-05-01
We present numerical studies of dipolar spin ice in the presence of a magnetic field slightly tilted away from the [111] axis. We find a first-order transition from a kagome ice to a q =X state when the external field is tilted toward the [11 2 ¯] direction. This is consistent with the anomalous critical scattering previously observed in the neutron scattering experiment on the spin ice material Ho2Ti2O7 in a tilted field [T. Fennell et al., Nat. Phys. 3, 566 (2007), 10.1038/nphys632]. We show that this ordering originates from the antiferromagnetic alignment of spin chains on the kagome planes. The residual entropy of the kagome ice is fully recovered. Our result captures the features observed in the experiments and points to the importance of the dipolar interaction in determining ordered states in the spin ice materials. We place our results in the context of recent susceptibility measurements on Dy2Ti2O7 , showing two features for a [111] field.
Superconductivity and spin excitations in orbitally ordered FeSe
NASA Astrophysics Data System (ADS)
Kreisel, Andreas; Mukherjee, Shantanu; Hirschfeld, P. J.; Andersen, B. M.
We provide a band-structure with low-energy properties consistent with recent photoemission and quantum oscillations measurements on the Fe-based superconductor FeSe, including a mean-field like orbital ordering in the dxz /dyz channel, and show that this model also accounts for the temperature dependence of the measured Knight shift and the spin-relaxation rate. An RPA calculation of the dynamical spin susceptibility yields spin excitations which are peaked at wave vector (π , 0) in the 1-Fe Brillouin zone, with a broad maximum at energies of order a few meV. Furthermore, the superconducting gap structure obtained from spin fluctuation theory exhibits nodes on the electron pockets, consistent with the 'V'-shaped density of states measured by tunneling spectroscopy on this material. The redistribution of spectral weight in the superconducting state creates a (π , 0) ''neutron resonance'' as seen in recent experiments. Comparing to various experimental results, we give predictions for further studies A.K. and B.M.A. acknowledge financial support from a Lundbeckfond fellowship (Grant No. A9318). P.J.H. was partially supported by the Department of Energy under Grant No. DE-FG02-05ER46236.
Magnetic order the iron spins in NdOFeAs
NASA Astrophysics Data System (ADS)
Chen, Ying; Lynn, J. W.; Li, J.; Li, G.; Chen, G. F.; Luo, J. L.; Wang, N. L.; Dai, Pengcheng; Dela Cruz, C.; Mook, H. A.
2009-03-01
Polarized and unpolarized powder neutron-diffraction measurements have been carried out to investigate the iron magnetic order in the parent compound of one of the highest Tc system, NdFeAsO. Antiferromagnetic order is observed below 141 K [1], which is in close proximity to the structural distortion observed in this material [2]. The magnetic structure consists of chains of parallel spins that are arranged antiparallel between chains, which is the same in-plane spin arrangement as observed in all the other iron oxypnictide materials. Nearest-neighbor spins along the c axis are antiparallel like LaFeAsO [3]. The ordered moment is 0.25 (7) μB, which is the smallest ordered moment found so far in these systems. [3pt] [1]Ying Chen, J. W. Lynn, J. Li, G. Li, G. F. Chen, J. L. Luo, N. L. Wang, Pengcheng Dai, C. dela Cruz and H. A. Mook, Phys. Rev. B 78, 064515 2008. [0pt] [2]Y. Qiu, W. Bao, Q. Huang, T. Yildirim, J. M. Simmons, M. A. Green, J.W. Lynn, Y.C. Gasparovic, J. Li, T. Wu, G. Wu, and X.H. Chen, arXiv:0806.2195 (Phys. Rev. Lett. accepted). [0pt] [3] C. dela Cruz, Q. Huang, J. W. Lynn, J. Li, W. Ratcliff II, J. L. Zarestky, H. A. Mook, G. F. Chen, J. L. Luo, N. L. Wang, and P. Dai, Nature 453, 899 (2008).
Magnetic Order and Transitions in the Spin-web Compound Cu3TeO6
NASA Astrophysics Data System (ADS)
Månsson, Martin; Prša, Krunoslav; Sugiyama, Jun; Andreica, Daniel; Luetkens, Hubertus; Berger, Helmuth
The spin-web compound Cu3TeO6, belongs to an intriguing group of materials where magnetism is governed by3d9 copper Cu2+ ions. This compound has been sparsely experimentally studied and we here present the first investigation of its local magnetic properties using muon-spin relaxation/rotation(μ+SR). Our results show a clear long-range 3D magnetic order below TN as indicated by clear zero-field (ZF) muon-precessions. At TN = 61.7K a very sharp transition is observed in the weak transverse-field (wTF) as well as ZF data. Contrary to suggestions by susceptibility measurements and inelastic neutron scattering, we find no evidence for either static or dynamic (on the time-scale of μ+SR) spin-correlations above TN.
Phase ordering dynamics in spin-1 ferromagnetic condensates
NASA Astrophysics Data System (ADS)
Williamson, Lewis; Blakie, Peter
2016-05-01
Spinor Bose-Einstein condensates present rich phase diagrams for exploring phase transitions between states with different symmetry properties. In this work we simulate the approach to equilibrium of a spin-1 condensate quenched from an unmagnetised phase to three different ferromagnetic phases. The three ferromagnetic phases have Z2, SO(2) and SO(3) symmetries respectively and possess different conservation laws. Following the quench, domains of magnetization form, with each domain making an independent choice of the symmetry breaking order parameter. These domains grow and compete for the global equilibrium state. We find that this growth follows universal scaling laws and identify the dynamic universality class for each of the three quenches. Polar-core spin-vortices play a crucial role in the phase ordering of the SO(2) system and we identify fractal structures in the domain patterns of the SO(2) and SO(3) systems. We acknowledge support from the Marsden Fund of New Zealand.
Quantum dot spin coherence governed by a strained nuclear environment.
Stockill, R; Le Gall, C; Matthiesen, C; Huthmacher, L; Clarke, E; Hugues, M; Atatüre, M
2016-01-01
The interaction between a confined electron and the nuclei of an optically active quantum dot provides a uniquely rich manifestation of the central spin problem. Coherent qubit control combines with an ultrafast spin-photon interface to make these confined spins attractive candidates for quantum optical networks. Reaching the full potential of spin coherence has been hindered by the lack of knowledge of the key irreversible environment dynamics. Through all-optical Hahn echo decoupling we now recover the intrinsic coherence time set by the interaction with the inhomogeneously strained nuclear bath. The high-frequency nuclear dynamics are directly imprinted on the electron spin coherence, resulting in a dramatic jump of coherence times from few tens of nanoseconds to the microsecond regime between 2 and 3 T magnetic field and an exponential decay of coherence at high fields. These results reveal spin coherence can be improved by applying large magnetic fields and reducing strain inhomogeneity. PMID:27615704
Chain-based order and quantum spin liquids in dipolar spin ice
NASA Astrophysics Data System (ADS)
McClarty, P. A.; Sikora, O.; Moessner, R.; Penc, K.; Pollmann, F.; Shannon, N.
2015-09-01
Recent experiments on the spin-ice material Dy2Ti2O7 suggest that the Pauling "ice entropy," characteristic of its classical Coulombic spin-liquid state, may be lost at low temperatures [Pomaranski et al., Nat. Phys. 9, 353 (2013), 10.1038/nphys2591]. However, despite nearly two decades of intensive study, the nature of the equilibrium ground state of spin ice remains uncertain. Here we explore how long-range dipolar interactions D , short-range exchange interactions, and quantum fluctuations combine to determine the ground state of dipolar spin ice. We identify the organizational principle that ordered ground states are selected from a set of "chain states" in which dipolar interactions are exponentially screened. Using both quantum and classical Monte Carlo simulation, we establish phase diagrams as a function of quantum tunneling g and temperature T , and find that only a very small gc≪D is needed to stabilize a quantum spin liquid ground state. We discuss the implications of these results for Dy2Ti2O7 .
Controlling Spin Ordering in Rare-Earth Perovskite Vanadates
NASA Astrophysics Data System (ADS)
Wagner, Nicholas; Rondinelli, James
We investigate the role and influence of local structure distortions on the antiferromagnetic spin ordering temperatures for large A-site radii RVO3 perovskites (R=Yb-La) using a combination of data analytics (DA) and density functional theory (DFT). First, mode crystallography is used to parameterize the structural phase space. Next, we identify the important local structural features that correlate strongly with the Néel temperatures (TN) using Pearson correlation coefficients. From this data, we then formulate a regression model using gradient boosted decision trees (GBDT) that returns the relative importance of each feature in predicting TN. Our analysis indicates that the amplitude of the subtle Jahn-Teller active mode, which leads to variations in the V-O bond lengths and angles, could be used as an effective structural control parameter to modify the spin ordering temperature. We then validate this data-driven structure-property relationship in artificial vanadate structures using TN based on both our GBDT model and a model Hamiltonian using DFT energies. This combined approach allows us to gauge the accuracy of existing physical models for the antiferromagnetic ordering in vanadates and opens possible strategies to design materials with targeted TN.
Spin excitations of ferronematic order in underdoped cuprate superconductors
Seibold, G.; Di Castro, C.; Grilli, M.; Lorenzana, J.
2014-01-01
High-temperature superconductors exhibit a characteristic hourglass-shaped spectrum of magnetic fluctuations which most likely contribute to the pairing glue in the cuprates. Recent neutron scattering experiments in strongly underdoped compounds have revealed a significant low energy anisotropy of these fluctuations which we explain by a model in which topological defects of the antiferromagnet clump to producing domain wall segments with ferronematic order. This state does not invoke global charge order but breaks C4 rotational and inversion symmetry. The incommensurability of the low doping charge-disordered state is in good agreement with experiment and interpolates smoothly with the incommensurability of the stripe phase at higher doping. Within linear spin-wave theory the dynamic structure factor is in very good agreement with inelastic neutron scattering data and can account for the observed energy dependent anisotropy. PMID:24936723
Dynamics of spin I=3/2 under spin-locking conditions in an ordered environment.
van der Maarel, J R; Jesse, W; Hancu, I; Woessner, D E
2001-08-01
We have derived approximate analytic solutions to the master equation describing the evolution of the spin I=3/2 density operator in the presence of a radio-frequency (RF) field and both static and fluctuating quadrupolar interactions. Spectra resulting from Fourier transformation of the evolutions of the on-resonance spin-locked magnetization into the various coherences display two satellite pairs and, in some cases, a central line. The central line is generally trimodal, consisting of a narrow component related to a slowly relaxing mode and two broad components pertaining to two faster relaxing modes. The rates of the fast modes are sensitive to slow molecular motion. Neither the amplitude nor the width of the narrow component is affected by the magnitude of the static coupling, whereas the corresponding features of the broad components depend in a rather complicated manner on the spin-lock field strength and static quadrupolar interaction. Under certain experimental conditions, the dependencies of the amplitudes on the dynamics are seen to vanish and the relaxation rates reduce to relatively simple expressions. One of the promising emerging features is the fact that the evolutions into the selectively detected quadrupolar spin polarization order and the rank-two double-quantum coherence do not exhibit a slowly relaxing mode and are particularly sensitive to slow molecular motion. Furthermore, these coherences can only be excited in the presence of a static coupling and this makes it possible to discern nuclei in anisotropic from those in isotropic environment. The feasibility of the spin-lock pulse sequences with limited RF power and a nonvanishing average electric field gradient has been demonstrated through experiments on sodium in a dense lyotropic DNA liquid crystal. PMID:11531352
NASA Astrophysics Data System (ADS)
Kim, Sang-Il; Kim, Dong-Jun; Seo, Min-Su; Park, Byong-Guk; Park, Seung-Young
2015-05-01
The dependence of the measured DC voltage on the non-magnetic material (NM) in NM/CoFeB and CoFeB/NM bilayers is studied under ferromagnetic resonance conditions in a TE011 resonant cavity. The directional change of the inverse spin Hall effect (ISHE) voltage VISHE for the stacking order of the bilayer can separate the pure VISHE and the anomalous Hall effect (AHE) voltage VAHE utilizing the method of addition and subtraction. The Ta and Ti NMs show a broad deviation of the spin Hall angle θISH, which originates from the AHE in accordance with the high resistivity of NMs. However, the Pt and Pd NMs show that the kinds of NMs with low resistivity are consistent with the previously reported θISH values. Therefore, the characteristics that NM should simultaneously satisfy to obtain a reasonable VISHE value in bilayer systems are large θISH and low resistivity.
Equilibrium pricing in an order book environment: Case study for a spin model
NASA Astrophysics Data System (ADS)
Meudt, Frederik; Schmitt, Thilo A.; Schäfer, Rudi; Guhr, Thomas
2016-07-01
When modeling stock market dynamics, the price formation is often based on an equilibrium mechanism. In real stock exchanges, however, the price formation is governed by the order book. It is thus interesting to check if the resulting stylized facts of a model with equilibrium pricing change, remain the same or, more generally, are compatible with the order book environment. We tackle this issue in the framework of a case study by embedding the Bornholdt-Kaizoji-Fujiwara spin model into the order book dynamics. To this end, we use a recently developed agent based model that realistically incorporates the order book. We find realistic stylized facts. We conclude for the studied case that equilibrium pricing is not needed and that the corresponding assumption of a "fundamental" price may be abandoned.
Spin and quadrupolar orders in the spin-1 bilinear-biquadratic model for iron-based superconductors
NASA Astrophysics Data System (ADS)
Luo, Cheng; Datta, Trinanjan; Yao, Dao-Xin
2016-06-01
Motivated by the recent experimental and theoretical progress of the magnetic properties in iron-based superconductors, we provide a comprehensive analysis of the extended spin-1 bilinear-biquadratic (BBQ) model on the square lattice. Using a variational approach at the mean-field level, we identify the existence of various magnetic phases, including conventional spin dipolar orders (ferro- and antiferromagnet), novel quadrupolar orders (spin nematic), and mixed dipolar-quadrupolar orders. In contrast to the regular Heisenberg model, the elementary excitations of the spin-1 BBQ model are described by the SU(3) flavor-wave theory. By fitting the experimental spin-wave dispersion, we determine the refined exchange couplings corresponding to the collinear antiferromagnetic iron pnictides. We also present the dynamic structure factors of both spin dipolar and quadrupolar components with connections to the future experiments.
Topological order in an exactly solvable 3D spin model
Bravyi, Sergey; Leemhuis, Bernhard; Terhal, Barbara M.
2011-04-15
Research highlights: RHtriangle We study exactly solvable spin model with six-qubit nearest neighbor interactions on a 3D face centered cubic lattice. RHtriangle The ground space of the model exhibits topological quantum order. RHtriangle Elementary excitations can be geometrically described as the corners of rectangular-shaped membranes. RHtriangle The ground space can encode 4g qubits where g is the greatest common divisor of the lattice dimensions. RHtriangle Logical operators acting on the encoded qubits are described in terms of closed strings and closed membranes. - Abstract: We study a 3D generalization of the toric code model introduced recently by Chamon. This is an exactly solvable spin model with six-qubit nearest-neighbor interactions on an FCC lattice whose ground space exhibits topological quantum order. The elementary excitations of this model which we call monopoles can be geometrically described as the corners of rectangular-shaped membranes. We prove that the creation of an isolated monopole separated from other monopoles by a distance R requires an operator acting on {Omega}(R{sup 2}) qubits. Composite particles that consist of two monopoles (dipoles) and four monopoles (quadrupoles) can be described as end-points of strings. The peculiar feature of the model is that dipole-type strings are rigid, that is, such strings must be aligned with face-diagonals of the lattice. For periodic boundary conditions the ground space can encode 4g qubits where g is the greatest common divisor of the lattice dimensions. We describe a complete set of logical operators acting on the encoded qubits in terms of closed strings and closed membranes.
Resonant-spin-ordering of vortex cores in interacting mesomagnets
NASA Astrophysics Data System (ADS)
Jain, Shikha
2013-03-01
The magnetic system of interacting vortex-state elements have a dynamically reconfigurable ground state characterized by different relative polarities and chiralities of the individual disks; and have a corresponding dynamically controlled spectrum of collective excitation modes that determine the microwave absorption of the crystal. The development of effective methods for dynamic control of the ground state in this vortex-type magnonic crystal is of interest both from fundamental and technological viewpoints. Control of vortex chirality has been demonstrated previously using various techniques; however, control and manipulation of vortex polarities remain challenging. In this work, we present a robust and efficient way of selecting the ground state configuration of interacting magnetic elements using resonant-spin-ordering approach. This is achieved by driving the system from the linear regime of constant vortex gyrations to the non-linear regime of vortex-core reversals at a fixed excitation frequency of one of the coupled modes. Subsequently reducing the excitation field to the linear regime stabilizes the system to a polarity combination whose resonant frequency is decoupled from the initialization frequency. We have utilized the resonant approach to transition between the two polarity combinations (parallel or antiparallel) in a model system of connected dot-pairs which may form the building blocks of vortex-based magnonic crystals. Taking a step further, we have extended the technique by studying many-particle system for its potential as spin-torque oscillators or logic devices. Work at Argonne was supported by the U. S. DOE, Office of BES, under Contract No. DE-AC02-06CH11357. This work was in part supported by grant DMR-1015175 from the U. S. National Science Foundation, by a Contract from the U.S. Army TARDEC and RDECOM.
Interaction induced staggered spin-orbit order in two-dimensional electron gas
Das, Tanmoy
2012-06-05
Decoupling spin and charge transports in solids is among the many prerequisites for realizing spin electronics, spin caloritronics, and spin-Hall effect. Beyond the conventional method of generating and manipulating spin current via magnetic knob, recent advances have expanded the possibility to optical and electrical method which are controllable both internally and externally. Yet, due to the inevitable presence of charge excitations and electrical polarizibility in these methods, the separation between spin and charge degrees of freedom of electrons remains a challenge. Here we propose and formulate an interaction induced staggered spin-orbit order as a new emergent phase of matter. We show that when some form of inherent spin-splitting via Rashba-type spin-orbit coupling renders two helical Fermi surfaces to become significantly nested, a Fermi surface instability arises. To lift this degeneracy, a spontaneous symmetry breaking spin-orbit density wave develops, causing a surprisingly large quasiparticle gapping with chiral electronic states, with no active charge excitations. Since the staggered spin-orbit order is associated with a condensation energy, quantified by the gap value, destroying such spin-orbit interaction costs sufficiently large perturbation field or temperature or de-phasing time. BiAg2 surface state is shown to be a representative system for realizing such novel spin-orbit interaction with tunable and large strength, and the spin-splitting is decoupled from charge excitations.
Kim, Sang-Il; Seo, Min-Su; Park, Seung-Young; Kim, Dong-Jun; Park, Byong-Guk
2015-05-07
The dependence of the measured DC voltage on the non-magnetic material (NM) in NM/CoFeB and CoFeB/NM bilayers is studied under ferromagnetic resonance conditions in a TE{sub 011} resonant cavity. The directional change of the inverse spin Hall effect (ISHE) voltage V{sub ISHE} for the stacking order of the bilayer can separate the pure V{sub ISHE} and the anomalous Hall effect (AHE) voltage V{sub AHE} utilizing the method of addition and subtraction. The Ta and Ti NMs show a broad deviation of the spin Hall angle θ{sub ISH}, which originates from the AHE in accordance with the high resistivity of NMs. However, the Pt and Pd NMs show that the kinds of NMs with low resistivity are consistent with the previously reported θ{sub ISH} values. Therefore, the characteristics that NM should simultaneously satisfy to obtain a reasonable V{sub ISHE} value in bilayer systems are large θ{sub ISH} and low resistivity.
Charge and spin order in one dimensional systems with long range Coulomb interaction
NASA Astrophysics Data System (ADS)
Belen Valenzuela, M.; Fratini, Simone; Baeriswyl, Dionys
2004-03-01
In this talk I present our results of studying a system of electrons on a one-dimensional lattice, interacting through long range Coulomb forces, by means of a variational technique which is the strong coupling analog of the Gutzwiller approach. For quarter filling we find that the effects of commensurability together with the strength of the interaction give rise to charge ordering as the ground state. When we add the spin degrees of freedom it is found that they are coupled by an antiferromagnetic kinetic exchange J, which turn out to be much smaller than the energy scale governing the charge degrees of freedom. Our results shed new light on the insulating phases of organic quasi-1D compounds where charge ordering sets in at high temperatures and coexists with spin ordering at low temperatures. We also present a phase diagram of interaction versus fillings where we identify three phases: weak charge density waves, Wigner crystal and Generalized Wigner crystal (solution of the Wigner crystal problem with the additional constraint for the electrons of living in the host lattice of the ions). Refs: B. Valenzuela et al. Phys. Rev. B, 68 (2003) 045112, S. Fratini et al. Contribution to the Michael J. Rice Special Issue of "Synthetic Metals" 2003, (cond-mat/0309450).
Dzyaloshinskii-Moriya Interaction and Spiral Order in Spin-orbit Coupled Optical Lattices
Gong, Ming; Qian, Yinyin; Yan, Mi; Scarola, V. W.; Zhang, Chuanwei
2015-01-01
We show that the recent experimental realization of spin-orbit coupling in ultracold atomic gases can be used to study different types of spin spiral order and resulting multiferroic effects. Spin-orbit coupling in optical lattices can give rise to the Dzyaloshinskii-Moriya (DM) spin interaction which is essential for spin spiral order. By taking into account spin-orbit coupling and an external Zeeman field, we derive an effective spin model in the Mott insulator regime at half filling and demonstrate that the DM interaction in optical lattices can be made extremely strong with realistic experimental parameters. The rich finite temperature phase diagrams of the effective spin models for fermions and bosons are obtained via classical Monte Carlo simulations. PMID:26014458
Influence of orbital nematic order on spin responses in Fe-based superconductors
NASA Astrophysics Data System (ADS)
Su, Yuehua; Zhang, Chao; Li, Tao
2016-05-01
Electronic nematicity is ubiquitous in Fe-based superconductors, but what the primary nematic order is and how the various nematic phenomena correlate with each other are still elusive. In this manuscript we study the physical consequence of the orbital nematic order on the spin correlations. We find that the orbital nematic order can drive a significant spin nematicity and can enhance the integrated intensity of the spin fluctuations. Our study shows that the orbital nematic order has strong effect on the spin correlations and it can not be taken as an unimportant secondary effect of the nematic state in Fe-based superconductors.
Critical competition between two distinct orbital-spin ordered states in perovskite vanadates
NASA Astrophysics Data System (ADS)
Fujioka, J.; Yasue, T.; Miyasaka, S.; Yamasaki, Y.; Arima, T.; Sagayama, H.; Inami, T.; Ishii, K.; Tokura, Y.
2010-10-01
We have investigated the spin/orbital phase diagram in the perovskite orthovanadate RVO3 ( R=Eu , Y, Dy, and Ho) by measurements of magnetization, dielectric constant, specific heat, Raman scattering spectra, and x-ray diffraction, focusing on the interplay between the V3d spin and the 4f moment of the R ion. The thermally induced phase transition between the C-type spin/G-type orbital ordered state and the G-type spin/C-type orbital ordered state is observed for Eu1-xYxVO3 (x=0-0.52) without 4f moment. By comparing this phase diagram with the spin/orbital ordering in TbVO3 , it is evident that the critical competition between the C-type spin/G-type orbital ordered phase and the G-type spin/C-type orbital ordered one depends not only on the GdFeO3 -type lattice distortion but also on the presence of the 4f moment of the R ion. The magnetic field induced phase transition of the spin/orbital ordering is achieved concomitantly with polarizing R4f moments for DyVO3 and HoVO3 . For DyVO3 , the G-type spin/C-type orbital ordered phase is switched to the C-type spin/G-type orbital ordered one by applying a moderate magnetic field around 3 T. By contrast, the G-type spin/C-type orbital ordering is rather favored under the magnetic field in HoVO3 . The results cannot be uniquely explained in terms of the exchange interaction between the V3d spin and the R -ion 4f moment. The coupling of the R4f moment polarization with the lattice distortion tied with the orbital ordering of the V3d sublattice may also be relevant to this field induced phase transition.
Surface spin-electron acoustic waves in magnetically ordered metals
NASA Astrophysics Data System (ADS)
Andreev, Pavel A.; Kuz'menkov, L. S.
2016-05-01
Degenerate plasmas with motionless ions show existence of three surface waves: the Langmuir wave, the electromagnetic wave, and the zeroth sound. Applying the separated spin evolution quantum hydrodynamics to half-space plasma, we demonstrate the existence of the surface spin-electron acoustic wave (SSEAW). We study dispersion of the SSEAW. We show that there is hybridization between the surface Langmuir wave and the SSEAW at rather small spin polarization. In the hybridization area, the dispersion branches are located close to each other. In this area, there is a strong interaction between these waves leading to the energy exchange. Consequently, generating the Langmuir waves with the frequencies close to hybridization area we can generate the SSEAWs. Thus, we report a method of creation of the spin-electron acoustic waves.
Damped spin waves in the intermediate ordered phases in Ni3V2O8
Ehlers, Georg; Podlesnyak, Andrey A.; Frontzek, Matthias D.; Pushkarev, A. V.; Shiryaev, Sergie V.; Barilo, Sergie
2015-06-09
Here, spin dynamics in the intermediate ordered phases (between 4 and 9 K) in Ni3V2O8 have been studied with inelastic neutron scattering. It is found that the spin waves are very diffuse, indicative of short lived correlations and the coexistence of paramagnetic moments with the long-range ordered state.
76 FR 53937 - Order of Succession for Government National Mortgage Association (GNMA)
Federal Register 2010, 2011, 2012, 2013, 2014
2011-08-30
... URBAN DEVELOPMENT Order of Succession for Government National Mortgage Association (GNMA) AGENCY: Office... Succession. SUMMARY: In this notice, the President of the Government National Mortgage Association (GNMA) designates the Order of Succession for GNMA. This Order of Succession supersedes all prior Orders...
Spatial confinement governs orientational order in patchy particles
NASA Astrophysics Data System (ADS)
Iwashita, Yasutaka; Kimura, Yasuyuki
2016-06-01
Orientational order in condensed matter plays a key role in determining material properties such as ferromagnetism, viscoelasticity or birefringence. We studied purely orientational ordering in closely-packed one-patch colloidal particles confined between flat substrates, where the particles can only rotate and are ordered via the sticky interaction between the patches. For the first time, we experimentally realized a rich variety of mesoscopic patterns through orientational ordering of colloids by controlling patch size and confinement thickness. The combination of experiment and numerical simulation reveals the decisive role of confinement: An ordered state(s) is selected from the (meta)stable options in bulk when it is commensurate with the system geometry and boundary conditions; otherwise, frustration induces a unique order. Our study offers a new means of systematic control over mesoscopic structures via orientational ordering in patchy particles. The system would also possess unique functionalities through the rotational response of the particles to external stimuli.
Spatial confinement governs orientational order in patchy particles
Iwashita, Yasutaka; Kimura, Yasuyuki
2016-01-01
Orientational order in condensed matter plays a key role in determining material properties such as ferromagnetism, viscoelasticity or birefringence. We studied purely orientational ordering in closely-packed one-patch colloidal particles confined between flat substrates, where the particles can only rotate and are ordered via the sticky interaction between the patches. For the first time, we experimentally realized a rich variety of mesoscopic patterns through orientational ordering of colloids by controlling patch size and confinement thickness. The combination of experiment and numerical simulation reveals the decisive role of confinement: An ordered state(s) is selected from the (meta)stable options in bulk when it is commensurate with the system geometry and boundary conditions; otherwise, frustration induces a unique order. Our study offers a new means of systematic control over mesoscopic structures via orientational ordering in patchy particles. The system would also possess unique functionalities through the rotational response of the particles to external stimuli. PMID:27264521
Absence of spin order in a two-dimensional orbital optical lattice
NASA Astrophysics Data System (ADS)
Zhou, Zhenyu; Liu, Vincent; Zhao, Erhai
2015-03-01
Mott insulators with both spin and orbital degeneracy are pertinent to a family of transition metal oxides. The intertwined spin and orbital fluctuations can lead to exotic phases such as quantum spin-orbital liquids. Here we consider two-component spin 1/2 fermionic atoms with strong repulsive interaction on the p-band of the square optical lattice. We derive the spin-orbital exchange for quarter filling of the p-band in the Mott limit, and show it frustrates the development of long range spin order. Exact diagonalization indicates a spin-disordered ground state with ferro-orbital order. The system dynamically decouples into individual Heisenberg spin chains, each realizing a Luttinger liquid accessible at higher temperatures compared to atoms confined to the s-band. Our model serves as an example of how orbital order enhances quantum fluctuations to prevent spin order and leads to dimension reduction in a quantum gas system. This work is supported by AFOSR FA9550-12-1-0079, NSF PHY-1205504, and ARO W911NF-11-1-0230.
Geometrical structure and spin order of Gd13 cluster
NASA Astrophysics Data System (ADS)
Yuan, H. K.; Chen, H.; Kuang, A. L.; Wu, B.
2011-09-01
The spin-polarized generalized gradient approximation to the density-functional theory has been used to determine the lowest energy structure, electronic structure, and magnetic property of Gd13 cluster. Our results show that the ionic bonding is combined with the covalent characteristics in stabilizing the Gd cluster. The ferrimagnetic icosahedron is found to be the lowest energy configuration, in which the centered Gd atom couples antiferromagnetically with the rest Gd atoms surrounding it. No spin non-collinear evidence has been detected in our calculations. It is identified that the local magnetic moments of Gd atom are about 8 μB regardless of geometrical structure. Finally, the comprehensive electronic structure analyses show that the indirect long-range magnetic coupling between the polarized 4f is mediated by the polarization of 5d, 6s, and 6p conduction electrons, which is the typical Ruderman-Kittel-Kasuya-Yosida interactions.
Ferrimagnetic ordering and spin entropy of field-dependent intermediate spins in Na0.82CoO2
NASA Astrophysics Data System (ADS)
Shu, G. J.; Chou, F. C.
2016-04-01
The peculiar field-dependent magnetism of Na0.82CoO2 has been investigated through an analysis of its dc and ac spin susceptibilities. To account for the easily activated narrow b2 g-a1 g gap of the crystal field for Co in the cobalt oxide layer, the spin-state transition of Co3 + (3 d6 ) between the low-spin (LS) state b2g 2a1g 0 of S =0 and the intermediate-spin (IS) state b2g 1a1g 1 of S =1 is thus seen as thermally activated and exhibits a Boltzmann distribution. The IS state of Co3 + within each √{13 }a hexagonal superlattice formed by the S =1 /2 state of the Co4 + ions appears randomly within each supercell and shows significant temperature and field dependence. The magnetic field is found to assist in pinning down the thermally activated state of Co3 + and swings the Boltzmann distribution weight toward a higher fraction of the IS state. The field dependence of the in-plane magnetic moment from the added number of S =1 spins is used to explain the origin of A -type antiferromagnetic (AF) ordering, particularly that the ferromagnetic (FM)-like behavior below TN at low field is actually a ferrimagnetic IS spin ordering of Co3 +.
Recoil velocity at second post-Newtonian order for spinning black hole binaries
NASA Astrophysics Data System (ADS)
Racine, Étienne; Buonanno, Alessandra; Kidder, Larry
2009-08-01
We compute the flux of linear momentum carried by gravitational waves emitted from spinning binary black holes at second post-Newtonian (2PN) order for generic orbits. In particular we provide explicit expressions of three new types of terms, namely, next-to-leading order spin-orbit terms at 1.5 post-Newtonian (1.5PN) order, spin-orbit tail terms at 2PN order, and spin-spin terms at 2PN order. Restricting ourselves to quasicircular orbits, we integrate the linear-momentum flux over time to obtain the recoil velocity as function of orbital frequency. We find that in the so-called superkick configuration the higher-order spin corrections can increase the recoil velocity up to a factor ˜3 with respect to the leading-order PN prediction. Whereas the recoil velocity computed in PN theory within the adiabatic approximation can accurately describe the early inspiral phase, we find that its fast increase during the late inspiral and plunge, and the arbitrariness in determining until when it should be trusted, makes the PN predictions for the total recoil not very accurate and robust. Nevertheless, the linear-momentum flux at higher PN orders can be employed to build more reliable resummed expressions aimed at capturing the nonperturbative effects until merger. Furthermore, we provide expressions valid for generic orbits, and accurate at 2PN order, for the energy and angular momentum carried by gravitational waves emitted from spinning binary black holes. Specializing to quasicircular orbits we compute the spin-spin terms at 2PN order in the expression for the evolution of the orbital frequency and found agreement with Mikóczi, Vasúth, and Gergely. We also verified that in the limit of extreme mass ratio our expressions for the energy and angular momentum fluxes match the ones of Tagoshi, Shibata, Tanaka, and Sasaki obtained in the context of black hole perturbation theory.
Transmission of spin waves in ordered FeRh epitaxial thin films
NASA Astrophysics Data System (ADS)
Usami, Takamasa; Suzuki, Ippei; Itoh, Mitsuru; Taniyama, Tomoyasu
2016-06-01
We report on B2-ordering dependence of magnetostatic surface spin waves in ferromagnetic FeRh at room temperature. Spin waves transmit over a distance longer than 21 μm in highly ordered FeRh alloys even with relatively large spin-orbit interaction. The long-range transmission likely arises from the induced Rh moments of the ordered FeRh due to ferromagnetic exchange interaction between Fe and Rh. The results indicate a potential of using FeRh in spintronic and magnonic applications by integrating with other fascinating magnetic characteristics of FeRh such as electric field induced magnetic phase transition.
Spin-controlled orbital motion in tightly focused high-order Laguerre-Gaussian beams.
Cao, Yongyin; Zhu, Tongtong; Lv, Haiyi; Ding, Weiqiang
2016-02-22
Spin angular momentum can contribute to both optical force and torque exerted on spheres. Orbit rate of spheres located in tightly focused LG beams with the same azimuthal mode index l is spin-controlled due to spin-orbit coupling. Laguerre-Gaussian beams with high-order azimuthal mode are used here to study the orbit rate of dielectric spheres. Orbit rates of spheres with varying sizes and refravtive indices are investigated as well as optical forces acting on spheres in LG beams with different azimuthal modes. These results would be much helpful to investigation on optical rotation and transfer of spin and orbital angular momentum. PMID:26906996
Government: Executive Order Brings Federal Agencies Under OSHA Rules.
ERIC Educational Resources Information Center
Chemical and Engineering News, 1980
1980-01-01
Outlined are implications for the execution of an executive order, effective July 1, 1980, requiring federal agencies to comply with the same occupational safety and health standards that private employers must meet. A brief history of prior attempts to put similar safeguards on federal facilities is provided. (CS)
TOPICAL REVIEW: Quantum spin nanotubes—frustration, competing orders and criticalities
NASA Astrophysics Data System (ADS)
Sakai, Tôru; Sato, Masahiro; Okamoto, Kiyomi; Okunishi, Kouichi; Itoi, Chigak
2010-10-01
Recent developments of theoretical studies on spin nanotubes are reviewed, especially focusing on the S = 1/2 three-leg spin tube. In contrast to the three-leg spin ladder, the tube has a spin gap in the case of the regular-triangle unit cell when the rung interaction is sufficiently large. The effective theory based on the Hubbard Hamiltonian indicates a quantum phase transition to a gapless spin liquid due to the lattice distortion to an isosceles triangle. This is also supported by the numerical diagonalization and the density matrix renormalization group analyses. Furthermore, combining analytical and numerical approaches, we reveal several novel magnetic-field-induced phenomena: Néel, dimer, chiral and/or inhomogeneous orders, a new mechanism for the magnetization plateau formation, and others. The recently synthesized spin tube materials are also briefly introduced.
Canonical Hamiltonian for an extended test body in curved spacetime: To quadratic order in spin
NASA Astrophysics Data System (ADS)
Vines, Justin; Kunst, Daniela; Steinhoff, Jan; Hinderer, Tanja
2016-03-01
We derive a Hamiltonian for an extended spinning test-body in a curved background spacetime, to quadratic order in the spin, in terms of three-dimensional position, momentum, and spin variables having canonical Poisson brackets. This requires a careful analysis of how changes of the spin supplementary condition are related to shifts of the body's representative worldline and transformations of the body's multipole moments, and we employ bitensor calculus for a precise framing of this analysis. We apply the result to the case of the Kerr spacetime and thereby compute an explicit canonical Hamiltonian for the test-body limit of the spinning two-body problem in general relativity, valid for generic orbits and spin orientations, to quadratic order in the test spin. This fully relativistic Hamiltonian is then expanded in post-Newtonian orders and in powers of the Kerr spin parameter, allowing comparisons with and extensions of the test-mass limits of available post-Newtonian results. Both the fully relativistic Hamiltonian and the results of its expansion can inform the construction of waveform models, especially effective-one-body models, for the analysis of gravitational waves from compact binaries.
Canonical Hamiltonian for an extended test body in curved spacetime: To quadratic order in spin
NASA Astrophysics Data System (ADS)
Vines, Justin; Kunst, Daniela; Steinhoff, Jan; Hinderer, Tanja
2016-05-01
We derive a Hamiltonian for an extended spinning test body in a curved background spacetime, to quadratic order in the spin, in terms of three-dimensional position, momentum, and spin variables having canonical Poisson brackets. This requires a careful analysis of how changes of the spin supplementary condition are related to shifts of the body's representative worldline and transformations of the body's multipole moments, and we employ bitensor calculus for a precise framing of this analysis. We apply the result to the case of the Kerr spacetime and thereby compute an explicit canonical Hamiltonian for the test-body limit of the spinning two-body problem in general relativity, valid for generic orbits and spin orientations, to quadratic order in the test spin. This fully relativistic Hamiltonian is then expanded in post-Newtonian orders and in powers of the Kerr spin parameter, allowing comparisons with the test-mass limits of available post-Newtonian results. Both the fully relativistic Hamiltonian and the results of its expansion can inform the construction of waveform models, especially effective-one-body models, for the analysis of gravitational waves from compact binaries.
Spin-squared Hamiltonian of next-to-leading order gravitational interaction
Steinhoff, Jan; Hergt, Steven; Schaefer, Gerhard
2008-11-15
The static, i.e., linear momentum independent, part of the next-to-leading order (NLO) gravitational spin(1)-spin(1) interaction Hamiltonian within the post-Newtonian (PN) approximation is calculated from a three-dimensional covariant ansatz for the Hamilton constraint. All coefficients in this ansatz can be uniquely fixed for black holes. The resulting Hamiltonian fits into the canonical formalism of Arnowitt, Deser, and Misner (ADM) and is given in their transverse-traceless (ADMTT) gauge. This completes the recent result for the momentum dependent part of the NLO spin(1)-spin(1) ADM Hamiltonian for binary black holes (BBH). Thus, all PN NLO effects up to quadratic order in spin for BBH are now given in Hamiltonian form in the ADMTT gauge. The equations of motion resulting from this Hamiltonian are an important step toward more accurate calculations of templates for gravitational waves.
Deciphering the rules governing assembly order of mammalian septin complexes.
Sellin, Mikael E; Sandblad, Linda; Stenmark, Sonja; Gullberg, Martin
2011-09-01
Septins are conserved GTP-binding proteins that assemble into lateral diffusion barriers and molecular scaffolds. Vertebrate genomes contain 9-17 septin genes that encode both ubiquitous and tissue-specific septins. Expressed septins may assemble in various combinations through both heterotypic and homotypic G-domain interactions. However, little is known regarding assembly states of mammalian septins and mechanisms directing ordered assembly of individual septins into heteromeric units, which is the focus of this study. Our analysis of the septin system in cells lacking or overexpressing selected septins reveals interdependencies coinciding with previously described homology subgroups. Hydrodynamic and single-particle data show that individual septins exist solely in the context of stable six- to eight-subunit core heteromers, all of which contain SEPT2 and SEPT6 subgroup members and SEPT7, while heteromers comprising more than six subunits also contain SEPT9. The combined data suggest a generic model for how the temporal order of septin assembly is homology subgroup-directed, which in turn determines the subunit arrangement of native heteromers. Because mammalian cells normally express multiple members and/or isoforms of some septin subgroups, our data also suggest that only a minor fraction of native heteromers are arranged as perfect palindromes. PMID:21737677
Quantum Effects in Higher-Order Correlators of a Quantum-Dot Spin Qubit
NASA Astrophysics Data System (ADS)
Bechtold, A.; Li, F.; Müller, K.; Simmet, T.; Ardelt, P.-L.; Finley, J. J.; Sinitsyn, N. A.
2016-07-01
We measure time correlators of a spin qubit in an optically active quantum dot beyond the second order. Such higher-order correlators are shown to be directly sensitive to pure quantum effects that cannot be explained within the classical framework. They allow direct determination of ensemble and quantum dephasing times, T2* and T2, using only repeated projective measurements and without the need for coherent spin control. Our method enables studies of purely quantum behavior in solid state systems, including tests of the Leggett-Garg type of inequalities that rule out local hidden variable interpretation of the quantum-dot spin dynamics.
Quantum Effects in Higher-Order Correlators of a Quantum-Dot Spin Qubit.
Bechtold, A; Li, F; Müller, K; Simmet, T; Ardelt, P-L; Finley, J J; Sinitsyn, N A
2016-07-01
We measure time correlators of a spin qubit in an optically active quantum dot beyond the second order. Such higher-order correlators are shown to be directly sensitive to pure quantum effects that cannot be explained within the classical framework. They allow direct determination of ensemble and quantum dephasing times, T_{2}^{*} and T_{2}, using only repeated projective measurements and without the need for coherent spin control. Our method enables studies of purely quantum behavior in solid state systems, including tests of the Leggett-Garg type of inequalities that rule out local hidden variable interpretation of the quantum-dot spin dynamics. PMID:27447523
48 CFR 252.251-7000 - Ordering from Government supply sources.
Code of Federal Regulations, 2012 CFR
2012-10-01
... supply sources. 252.251-7000 Section 252.251-7000 Federal Acquisition Regulations System DEFENSE... CLAUSES Text of Provisions And Clauses 252.251-7000 Ordering from Government supply sources. As prescribed in 251.107, use the following clause: Ordering From Government Supply Sources (AUG 2012) (a)...
48 CFR 252.251-7000 - Ordering from Government supply sources.
Code of Federal Regulations, 2013 CFR
2013-10-01
... supply sources. 252.251-7000 Section 252.251-7000 Federal Acquisition Regulations System DEFENSE... CLAUSES Text of Provisions And Clauses 252.251-7000 Ordering from Government supply sources. As prescribed in 251.107, use the following clause: Ordering From Government Supply Sources (AUG 2012) (a)...
Hidden order in spin-liquid Gd₃Ga₅O₁₂.
Paddison, Joseph A M; Jacobsen, Henrik; Petrenko, Oleg A; Fernández-Díaz, Maria Teresa; Deen, Pascale P; Goodwin, Andrew L
2015-10-01
Frustrated magnetic materials are promising candidates for new states of matter because lattice geometry suppresses conventional magnetic dipole order, potentially allowing "hidden" order to emerge in its place. A model of a hidden-order state at the atomic scale is difficult to deduce because microscopic probes are not directly sensitive to hidden order. Here, we develop such a model of the spin-liquid state in the canonical frustrated magnet gadolinium gallium garnet (Gd3Ga5O12). We show that this state exhibits a long-range hidden order in which multipoles are formed from 10-spin loops. The order is a consequence of the interplay between antiferromagnetic spin correlations and local magnetic anisotropy, which allows it to be indirectly observed in neutron-scattering experiments. PMID:26450205
High-order moments of spin-orbit energy in a multielectron configuration.
Na, Xieyu; Poirier, M
2016-07-01
In order to analyze the energy-level distribution in complex ions such as those found in warm dense plasmas, this paper provides values for high-order moments of the spin-orbit energy in a multielectron configuration. Using second-quantization results and standard angular algebra or fully analytical expressions, explicit values are given for moments up to 10th order for the spin-orbit energy. Two analytical methods are proposed, using the uncoupled or coupled orbital and spin angular momenta. The case of multiple open subshells is considered with the help of cumulants. The proposed expressions for spin-orbit energy moments are compared to numerical computations from Cowan's code and agree with them. The convergence of the Gram-Charlier expansion involving these spin-orbit moments is analyzed. While a spectrum with infinitely thin components cannot be adequately represented by such an expansion, a suitable convolution procedure ensures the convergence of the Gram-Charlier series provided high-order terms are accounted for. A corrected analytical formula for the third-order moment involving both spin-orbit and electron-electron interactions turns out to be in fair agreement with Cowan's numerical computations. PMID:27575229
High-order moments of spin-orbit energy in a multielectron configuration
NASA Astrophysics Data System (ADS)
Na, Xieyu; Poirier, M.
2016-07-01
In order to analyze the energy-level distribution in complex ions such as those found in warm dense plasmas, this paper provides values for high-order moments of the spin-orbit energy in a multielectron configuration. Using second-quantization results and standard angular algebra or fully analytical expressions, explicit values are given for moments up to 10th order for the spin-orbit energy. Two analytical methods are proposed, using the uncoupled or coupled orbital and spin angular momenta. The case of multiple open subshells is considered with the help of cumulants. The proposed expressions for spin-orbit energy moments are compared to numerical computations from Cowan's code and agree with them. The convergence of the Gram-Charlier expansion involving these spin-orbit moments is analyzed. While a spectrum with infinitely thin components cannot be adequately represented by such an expansion, a suitable convolution procedure ensures the convergence of the Gram-Charlier series provided high-order terms are accounted for. A corrected analytical formula for the third-order moment involving both spin-orbit and electron-electron interactions turns out to be in fair agreement with Cowan's numerical computations.
Félix, Gautier; Nicolazzi, William; Salmon, Lionel; Molnár, Gábor; Perrier, Marine; Maurin, Guillaume; Larionova, Joulia; Long, Jérôme; Guari, Yannick; Bousseksou, Azzedine
2013-06-01
We analyzed the size effect on a first-order spin transition governed by elastic interactions. This study was performed in the framework of a nonextensive thermodynamic core-shell model. When decreasing the particle size, differences in surface energies between the two phases lead to the shrinking of the thermal hysteresis width, the lowering of the transition temperature, and the increase of residual fractions at low temperature, in good agreement with recent experimental observations on spin transition nanomaterials. On the other hand, a modification of the particle-matrix interface may allow for the existence of the hysteresis loop even at very low sizes. In addition, an unexpected reopening of the hysteresis, when the size decreases, is also possible due to the hardening of the nanoparticles at very small sizes, which we deduced from the size dependence of the Debye temperature of a series of coordination nanoparticles. PMID:25167512
NASA Astrophysics Data System (ADS)
Félix, Gautier; Nicolazzi, William; Salmon, Lionel; Molnár, Gábor; Perrier, Marine; Maurin, Guillaume; Larionova, Joulia; Long, Jérôme; Guari, Yannick; Bousseksou, Azzedine
2013-06-01
We analyzed the size effect on a first-order spin transition governed by elastic interactions. This study was performed in the framework of a nonextensive thermodynamic core-shell model. When decreasing the particle size, differences in surface energies between the two phases lead to the shrinking of the thermal hysteresis width, the lowering of the transition temperature, and the increase of residual fractions at low temperature, in good agreement with recent experimental observations on spin transition nanomaterials. On the other hand, a modification of the particle-matrix interface may allow for the existence of the hysteresis loop even at very low sizes. In addition, an unexpected reopening of the hysteresis, when the size decreases, is also possible due to the hardening of the nanoparticles at very small sizes, which we deduced from the size dependence of the Debye temperature of a series of coordination nanoparticles.
Next-to-leading order gravitational spin-orbit coupling in an effective field theory approach
Levi, Michele
2010-11-15
We use an effective field theory (EFT) approach to calculate the next-to-leading order (NLO) gravitational spin-orbit interaction between two spinning compact objects. The NLO spin-orbit interaction provides the most computationally complex sector of the NLO spin effects, previously derived within the EFT approach. In particular, it requires the inclusion of nonstationary cubic self-gravitational interaction, as well as the implementation of a spin supplementary condition (SSC) at higher orders. The EFT calculation is carried out in terms of the nonrelativistic gravitational field parametrization, making the calculation more efficient with no need to rely on automated computations, and illustrating the coupling hierarchy of the different gravitational field components to the spin and mass sources. Finally, we show explicitly how to relate the EFT derived spin results to the canonical results obtained with the Arnowitt-Deser-Misner (ADM) Hamiltonian formalism. This is done using noncanonical transformations, required due to the implementation of covariant SSC, as well as canonical transformations at the level of the Hamiltonian, with no need to resort to the equations of motion or the Dirac brackets.
Phase transitions and charge ordering in a square spin ice model with conserved monopole density
NASA Astrophysics Data System (ADS)
Xie, Yunlong; Zhou, Xiaohui; Liu, Jun-Ming
2015-03-01
Artificial spin ices represent a class of highly interested frustrated magnetic systems under intensive investigations for fascinating ground states and thermodynamics/dynamics of spin excitations in recent years. As one of these issues, magnetic charge ordering and the corresponding phase transitions in the two-dimensional system are emerging topics in condensed matter physics. In this work, we investigate all the monopole-ordered phases of the square spin ice model using the conserved monopole density algorithm. In low monopole density (ρ ~ 0), the Coulomb potential determines the monopoles' dynamics. We test the Coulomb's law in a two-dimension lattice and justify the monopole dimerization which is quite different from the three-dimensional pyrochlore spin ice. These monopole dimers are charge neutral, and the interactions between them have also been investigated using our algorithm. In the cases of high monopole density (ρ ~ 1), the system is similar to the dipolar kagome spin ice model, and our simulation results show that there exists an intermediate phase between the paramagnetic phase and the ordered magnetic phase. Such intermediate phase can be distinguished by the order of magnetic charges. In a cooling process, the system undergoes a two-stage magnetic phase transition before freezing to the long range magnetic ordered phase via a staggered charge ordering. Furthermore, a liquefaction process of monopole dimers can be justified upon the increasing effective internal pressure in the isothermal condition.
Spin-Lattice-Coupled Order in Heisenberg Antiferromagnets on the Pyrochlore Lattice
NASA Astrophysics Data System (ADS)
Aoyama, Kazushi; Kawamura, Hikaru
2016-06-01
Effects of local lattice distortions on the spin ordering are investigated for the antiferromagnetic classical Heisenberg model on the pyrochlore lattice. It is found by Monte Carlo simulations that the spin-lattice coupling (SLC) originating from site phonons induces a first-order transition into two different types of collinear magnetic ordered states. The state realized at the stronger SLC is cubic symmetric characterized by the magnetic (1/2 ,1/2 ,1/2 ) Bragg peaks, while that at the weaker SLC is tetragonal symmetric characterized by the (1,1,0) ones, each accompanied by the commensurate local lattice distortions. Experimental implications to chromium spinels are discussed.
Rusakova, Irina L; Krivdin, Leonid B
2013-11-01
A double perturbation theory (DPT) at the second order level of approximation formalism has been applied to examine the dihedral angle dependence of the Fermi-contact (FC) contribution to nuclear spin-spin coupling constants. The unperturbed wave function of the ground state in DPT was approximated by the Hartree-Fock Slater determinant, while the excited states were treated as the single excited determinants. An analytical expression relating the FC term of vicinal proton-proton spin-spin coupling constants across the aliphatic single carbon-carbon bond to the dihedral angle describing inner rotation around the C-C bond in the ten-electron ten-orbital moiety H-C-C-H has been derived and analyzed. In particular, it has been shown that extrema of (3)J(H,H) are observed at φ = πn, n = 0, ±1, ±2,…, which provides a theoretical background of a well-known semiempirical Karplus equation. PMID:24071769
Charge-ordering cascade with spin-orbit Mott dimer states in metallic iridium ditelluride.
Ko, K-T; Lee, H-H; Kim, D-H; Yang, J-J; Cheong, S-W; Eom, M J; Kim, J S; Gammag, R; Kim, K-S; Kim, H-S; Kim, T-H; Yeom, H-W; Koo, T-Y; Kim, H-D; Park, J-H
2015-01-01
Spin-orbit coupling results in technologically-crucial phenomena underlying magnetic devices like magnetic memories and energy-efficient motors. In heavy element materials, the strength of spin-orbit coupling becomes large to affect the overall electronic nature and induces novel states such as topological insulators and spin-orbit-integrated Mott states. Here we report an unprecedented charge-ordering cascade in IrTe2 without the loss of metallicity, which involves localized spin-orbit Mott states with diamagnetic Ir(4+)-Ir(4+) dimers. The cascade in cooling, uncompensated in heating, consists of first order-type consecutive transitions from a pure Ir(3+) phase to Ir(3+)-Ir(4+) charge-ordered phases, which originate from Ir 5d to Te 5p charge transfer involving anionic polymeric bond breaking. Considering that the system exhibits superconductivity with suppression of the charge order by doping, analogously to cuprates, these results provide a new electronic paradigm of localized charge-ordered states interacting with itinerant electrons through large spin-orbit coupling. PMID:26059464
3 CFR 13494 - Executive Order 13494 of January 30, 2009. Economy in Government Contracting
Code of Federal Regulations, 2010 CFR
2010-01-01
... 3 The President 1 2010-01-01 2010-01-01 false Executive Order 13494 of January 30, 2009. Economy... 13494 of January 30, 2009 EO 13494 Economy in Government Contracting By the authority vested in me as... promote economy and efficiency in Government contracting, certain costs that are not directly related...
Nearest-Neighbor Repulsion and Competing Charge and Spin Order in the Extended Hubbard Model.
NASA Astrophysics Data System (ADS)
Bahman, Davoudi; Tremblay, A.-M. S.
2006-03-01
We generalize the Two-Particle Self-Consistent (TPSC) approach to study the extended Hubbard model where the nearest-neighbor interaction V is present in addition to the local interaction U. Our results are in good agreement with available Quantum Monte-Carlo results over the whole range of density n up to intermediate coupling. As a function of U, V and n we observe different kinds of charge and spin orders, like commensurate/incommensurate charge and spin density wave, phase separation, and ferromagnetic order. For attractive V superconductivity could exist in the regions where the other types of charge and spin orders do not dominate. Ref.: B. Davoudi and A.-M.S. Tremblay, cond-mat/0509707
Enhanced Ferroelectric Polarization by Induced Dy Spin Order in Multiferroic DyMnO{sub 3}
Prokhnenko, O.; Landsgesell, S.; Aliouane, N.; Argyriou, D. N.; Feyerherm, R.; Dudzik, E.
2007-02-02
Neutron powder diffraction and single crystal x-ray resonant magnetic scattering measurements suggest that Dy plays an active role in enhancing the ferroelectric polarization in multiferroic DyMnO{sub 3} above T{sub N}{sup Dy}=6.5 K. We observe the evolution of an incommensurate ordering of Dy moments with the same periodicity as the Mn spiral ordering. It closely tracks the evolution of the ferroelectric polarization. Below T{sub N}{sup Dy}, where Dy spins order commensurately, the polarization decreases to values similar for those of TbMnO{sub 3}. The higher P{sub s} found just above T{sub N}{sup Dy} arises from the contribution of Dy spins so as to effectively increase the amplitude of the Mn spin spiral.
NASA Astrophysics Data System (ADS)
Pürrer, Michael
2016-03-01
I provide a frequency domain reduced order model (ROM) for the aligned-spin effective-one-body model "SEOBNRv2" for data analysis with second- and third-generation ground-based gravitational wave (GW) detectors. SEOBNRv2 models the dominant mode of the GWs emitted by the coalescence of black hole binaries. The large physical parameter space (dimensionless spins -1 ≤χi≤0.99 and symmetric mass ratios 0.01 ≤η ≤0.25 ) requires sophisticated reduced order modeling techniques, including patching in the parameter space and in frequency. I find that the time window over which the inspiral-plunge and the merger-ringdown waveform in SEOBNRv2 are connected has a discontinuous dependence on the parameters when the spin parameter χ =0.8 or the symmetric mass ratio η ˜0.083 . This discontinuity increases resolution requirements for the ROM. The ROM can be used for compact binary systems with total masses of 2 M⊙ or higher for the Advanced LIGO design sensitivity and a 10 Hz lower cutoff frequency. The ROM has a worst mismatch against SEOBNRv2 of ˜1 %, but in general mismatches are better than ˜0.1 %. The ROM is crucial for key data analysis applications for compact binaries, such as GW searches and parameter estimation carried out within the LIGO Scientific Collaboration.
Anisotropy: Spin order and magnetization of single-crystalline Cu4(OH) 6FBr barlowite
NASA Astrophysics Data System (ADS)
Han, Tian-Heng; Isaacs, Eric D.; Schlueter, John A.; Singleton, John
2016-06-01
Despite decades-long fascination, the difficulty of maintaining high lattice symmetry in frustrated nonbipartite S =1/2 materials that can also be made into high-quality single crystals has been a persistent challenge. Here we report magnetization studies of a single-crystal sample of barlowite, Cu4(OH) 6 FBr , which has a geometrically perfect kagome motif. At T ≤4.2 K and 35 ≤μ0H ≤65 T, the interlayer spins are fully polarized, and the kagome-intrinsic magnetization is consistent with a Heisenberg model having J /kB=-180 K. Several field-driven anomalies are observed, having varied scalings with temperature. At an applied field, kagome disorder caused by the interlayer spins is smaller than that in herbertsmithite. At T ≤ 15 K, the bulk magnetic moment comes from the interlayer spins. An almost coplanar spin order suggests that the magnitude of in-plane Dzyaloshinskii-Moriya interaction is smaller than 0.006(6) J . On the other hand, the possibility of a spin-liquid state in the kagome lattice coexisting with ordered interlayer spins is left open.
Refrustration and competing orders in the prototypical Dy2Ti2O7 spin ice material
NASA Astrophysics Data System (ADS)
Henelius, P.; Lin, T.; Enjalran, M.; Hao, Z.; Rau, J. G.; Altosaar, J.; Flicker, F.; Yavors'kii, T.; Gingras, M. J. P.
2016-01-01
Spin ices, frustrated magnetic materials analogous to common water ice, have emerged over the past 15 years as exemplars of high frustration in three dimensions. Recent experimental developments aimed at interrogating anew the low-temperature properties of these systems, in particular whether the predicted transition to long-range order occurs, behoove researchers to scrutinize our current dipolar spin ice model description of these materials. In this work, we do so by combining extensive Monte Carlo simulations and mean-field theory calculations to analyze data from previous magnetization, diffuse neutron scattering, and specific-heat measurements on the paradigmatic Dy2Ti2O7 spin ice material. In this work, we also reconsider the possible importance of the nuclear specific heat Cnuc in Dy2Ti2O7 . We find that Cnuc is not entirely negligible below a temperature ˜0.5 K and must therefore be taken into account in a quantitative analysis of the calorimetric data of this compound below that temperature. We find that in this material, small effective spin-spin exchange interactions compete with the magnetostatic dipolar interaction responsible for the main spin ice phenomenology. This causes an unexpected "refrustration" of the long-range order that would be expected from the incompletely self-screened dipolar interaction and which positions the material at the boundary between two competing classical long-range-ordered ground states. This allows for the manifestation of new physical low-temperature phenomena in Dy2Ti2O7 , as exposed by recent specific-heat measurements. We show that among the four most likely causes for the observed upturn of the specific heat at low temperature [an exchange-induced transition to long-range order, quantum non-Ising (transverse) terms in the effective spin Hamiltonian, the nuclear hyperfine contribution, and random disorder], only the last appears to be reasonably able to explain the calorimetric data.
Quantum size effects in competing charge and spin orderings of dangling bond wires on Si(001)
Lee, Ji Young; Cho, Jun-Hyung; Zhang, Zhenyu
2009-01-01
Using spin-polarized density-functional theory calculations, we investigate the competition between charge and spin orderings in dangling-bond DB wires of increasing lengths fabricated on an H-terminated Si 001 surface. For wires containing less than ten DBs as studied in recent experiments, we find antiferromagnetic AF ordering to be energetically much more favorable than charge ordering. The energy preference of AF ordering shrinks in an oscillatory way as the wire length increases and preserves its sign even for DB wires of infinite length. The oscillatory behavior can be attributed to quantum size effects as the DB electrons fill discrete quantum levels. The predicted AF ordering is in startling contrast with the prevailing picture of charge ordering due to Jahn-Teller distortion or Peierls instability for wires of finite or infinite lengths, respectively.
Chamati, Hassan; Romano, Silvano
2014-08-01
At low temperatures, some lattice spin models with simple ferromagnetic or antiferromagnetic interactions (for example, nearest-neighbor interaction being isotropic in spin space on a bipartite three-dimensional lattice) produce orientationally ordered phases exhibiting nematic (second-rank) order, in addition to the primary first-rank one; on the other hand, in the literature, they have been rather seldom investigated in this respect. Here we study the thermodynamic properties of a three-dimensional model with dipolar-like interaction. Its ground state is found to exhibit full orientational order with respect to a suitably defined staggered magnetization (polarization), but no nematic second-rank order. Extensive Monte Carlo simulations, in conjunction with finite-size scaling analysis, have been used for characterizing its critical behavior; on the other hand, it has been found that nematic order does indeed set in at low temperatures, via a mechanism of order by disorder. PMID:25215748
Magnetic-charge ordering and phase transitions in monopole-conserved square spin ice
Xie, Y.-L.; Du, Z.-Z.; Yan, Z.-B.; Liu, J.-M.
2015-01-01
Magnetic-charge ordering and corresponding magnetic/monopole phase transitions in spin ices are the emergent topics of condensed matter physics. In this work, we investigate a series of magnetic-charge (monopole) phase transitions in artificial square spin ice model using the conserved monopole density algorithm. It is revealed that the dynamics of low monopole density lattices is controlled by the effective Coulomb interaction and the Dirac string tension, leading to the monopole dimerization which is quite different from the dynamics of three-dimensional pyrochlore spin ice. The condensation of the monopole dimers into monopole crystals with staggered magnetic-charge order can be predicted clearly. For the high monopole density cases, the lattice undergoes two consecutive phase transitions from high-temperature paramagnetic/charge-disordered phase into staggered charge-ordered phase before eventually toward the long-range magnetically-ordered phase as the ground state which is of staggered charge order too. A phase diagram over the whole temperature-monopole density space, which exhibits a series of emergent spin and monopole ordered states, is presented. PMID:26511870
Magnetic-charge ordering and phase transitions in monopole-conserved square spin ice
NASA Astrophysics Data System (ADS)
Xie, Y.-L.; Du, Z.-Z.; Yan, Z.-B.; Liu, J.-M.
2015-10-01
Magnetic-charge ordering and corresponding magnetic/monopole phase transitions in spin ices are the emergent topics of condensed matter physics. In this work, we investigate a series of magnetic-charge (monopole) phase transitions in artificial square spin ice model using the conserved monopole density algorithm. It is revealed that the dynamics of low monopole density lattices is controlled by the effective Coulomb interaction and the Dirac string tension, leading to the monopole dimerization which is quite different from the dynamics of three-dimensional pyrochlore spin ice. The condensation of the monopole dimers into monopole crystals with staggered magnetic-charge order can be predicted clearly. For the high monopole density cases, the lattice undergoes two consecutive phase transitions from high-temperature paramagnetic/charge-disordered phase into staggered charge-ordered phase before eventually toward the long-range magnetically-ordered phase as the ground state which is of staggered charge order too. A phase diagram over the whole temperature-monopole density space, which exhibits a series of emergent spin and monopole ordered states, is presented.
Magnetic-charge ordering and phase transitions in monopole-conserved square spin ice.
Xie, Y-L; Du, Z-Z; Yan, Z-B; Liu, J-M
2015-01-01
Magnetic-charge ordering and corresponding magnetic/monopole phase transitions in spin ices are the emergent topics of condensed matter physics. In this work, we investigate a series of magnetic-charge (monopole) phase transitions in artificial square spin ice model using the conserved monopole density algorithm. It is revealed that the dynamics of low monopole density lattices is controlled by the effective Coulomb interaction and the Dirac string tension, leading to the monopole dimerization which is quite different from the dynamics of three-dimensional pyrochlore spin ice. The condensation of the monopole dimers into monopole crystals with staggered magnetic-charge order can be predicted clearly. For the high monopole density cases, the lattice undergoes two consecutive phase transitions from high-temperature paramagnetic/charge-disordered phase into staggered charge-ordered phase before eventually toward the long-range magnetically-ordered phase as the ground state which is of staggered charge order too. A phase diagram over the whole temperature-monopole density space, which exhibits a series of emergent spin and monopole ordered states, is presented. PMID:26511870
Levi, Michele; Steinhoff, Jan E-mail: jan.steinhoff@ist.utl.pt
2014-12-01
The next-to-next-to-leading order spin1-spin2 potential for an inspiralling binary, that is essential for accuracy to fourth post-Newtonian order, if both components in the binary are spinning rapidly, has been recently derived independently via the ADM Hamiltonian and the Effective Field Theory approaches, using different gauges and variables. Here we show the complete physical equivalence of the two results, thereby we first prove the equivalence of the ADM Hamiltonian and the Effective Field Theory approaches at next-to-next-to-leading order with the inclusion of spins. The main difficulty in the spinning sectors, which also prescribes the manner in which the comparison of the two results is tackled here, is the existence of redundant unphysical spin degrees of freedom, associated with the spin gauge choice of a point within the extended spinning object for its representative worldline. After gauge fixing and eliminating the unphysical degrees of freedom of the spin and its conjugate at the level of the action, we arrive at curved spacetime generalizations of the Newton-Wigner variables in closed form, which can also be used to obtain further Hamiltonians, based on an Effective Field Theory formulation and computation. Finally, we make use of our validated result to provide gauge invariant relations among the binding energy, angular momentum, and orbital frequency of an inspiralling binary with generic compact spinning components to fourth post-Newtonian order, including all known sectors up to date.
HfMnSb2 : A Metal-Ordered NiAs-type Pnictide with a Conical Spin Order.
Murakami, Taito; Yamamoto, Takafumi; Tassel, Cédric; Takatsu, Hiroshi; Ritter, Clemens; Ajiro, Yoshitami; Kageyama, Hiroshi
2016-08-16
The NiAs-type structure is one of the most common structures in solids, but metal order has been almost exclusively limited to chalcogenides. The synthesis of HfMnSb2 is reported with a novel metal-ordered NiAs-type structure. HfMnSb2 undergoes a conical spin order below 270 K, in marked contrast to conventional magnetic order observed in NiAs-type pnictides. We argue that the layered arrangement of Hf and Mn makes it a quasi 2D magnet, where the Mn layers with localized magnetic moments (Mn(2+) ; S=5/2) can interact only through RKKY interactions, instead of metal-metal bonding that is otherwise dominant for typical NiAs-type pnictides. This result suggests that controlling order-disorder in NiAs-type pnictides enables a study of 2D-to-3D crossover behavior in itinerant magnetic system. PMID:27355989
48 CFR 1480.502 - Order of precedence for use of Government supply sources.
Code of Federal Regulations, 2014 CFR
2014-10-01
... 48 Federal Acquisition Regulations System 5 2014-10-01 2014-10-01 false Order of precedence for use of Government supply sources. 1480.502 Section 1480.502 Federal Acquisition Regulations System DEPARTMENT OF THE INTERIOR INDIAN AFFAIRS SUPPLEMENT ACQUISITIONS UNDER THE BUY INDIAN ACT Procedures 1480.502 Order of precedence for use of...
Spin-Lattice Order in One-Dimensional Conductors: Beyond the RKKY Effect.
Schecter, Michael; Rudner, Mark S; Flensberg, Karsten
2015-06-19
We investigate magnetic order in a lattice of classical spins coupled to an isotropic gas of one-dimensional conduction electrons via local exchange interactions. The frequently discussed Ruderman-Kittel-Kasuya-Yosida effective exchange model for this system predicts that spiral order is always preferred. Here we consider the problem nonperturbatively, and find that such order vanishes above a critical value of the exchange coupling that depends strongly on the lattice spacing. The critical coupling tends to zero as the lattice spacing becomes commensurate with the Fermi wave vector, signaling the breakdown of the perturbative Ruderman-Kittel-Kasuya-Yosida picture, and spiral order, even at weak coupling. We provide the exact phase diagram for arbitrary exchange coupling and lattice spacing, and discuss its stability. Our results shed new light on the problem of utilizing a spiral spin-lattice state to drive a one-dimensional superconductor into a topological phase. PMID:26197005
Jung, Yousung; Lochan, Rohini C.; Dutoi, Anthony D.; Head-Gordon, Martin
2004-08-02
A simplified approach to treating the electron correlation energy is suggested in which only the alpha-beta component of the second order Moller-Plesset energy is evaluated, and then scaled by an empirical factor which is suggested to be 1.3. This scaled opposite spin second order energy (SOS-MP2) yields results for relative energies and derivative properties that are statistically improved over the conventional MP2 method. Furthermore, the SOS-MP2 energy can be evaluated without the 5th order computational steps associated with MP2 theory, even without exploiting any spatial locality. A 4th order algorithm is given for evaluating the opposite spin MP2 energy using auxiliary basis expansions, and a Laplace approach, and timing comparisons are given.
Spin-Lattice Order in One-Dimensional Conductors: Beyond the RKKY Effect
NASA Astrophysics Data System (ADS)
Schecter, Michael; Rudner, Mark S.; Flensberg, Karsten
2015-06-01
We investigate magnetic order in a lattice of classical spins coupled to an isotropic gas of one-dimensional conduction electrons via local exchange interactions. The frequently discussed Ruderman-Kittel-Kasuya-Yosida effective exchange model for this system predicts that spiral order is always preferred. Here we consider the problem nonperturbatively, and find that such order vanishes above a critical value of the exchange coupling that depends strongly on the lattice spacing. The critical coupling tends to zero as the lattice spacing becomes commensurate with the Fermi wave vector, signaling the breakdown of the perturbative Ruderman-Kittel-Kasuya-Yosida picture, and spiral order, even at weak coupling. We provide the exact phase diagram for arbitrary exchange coupling and lattice spacing, and discuss its stability. Our results shed new light on the problem of utilizing a spiral spin-lattice state to drive a one-dimensional superconductor into a topological phase.
Topological frustration in graphene nanoflakes: magnetic order and spin logic devices.
Wang, Wei L; Yazyev, Oleg V; Meng, Sheng; Kaxiras, Efthimios
2009-04-17
Magnetic order in graphene-related structures can arise from size effects or from topological frustration. We introduce a rigorous classification scheme for the types of finite graphene structures (nanoflakes) which lead to large net spin or to antiferromagnetic coupling between groups of electron spins. Based on this scheme, we propose specific examples of structures that can serve as the fundamental (NOR and NAND) logic gates for the design of high-density ultrafast spintronic devices. We demonstrate, using ab initio electronic structure calculations, that these gates can in principle operate at room temperature with very low and correctable error rates. PMID:19518670
Magnetic order and spin excitations in the Kitaev-Heisenberg model on a honeycomb lattice
NASA Astrophysics Data System (ADS)
Vladimirov, A. A.; Ihle, D.; Plakida, N. M.
2016-06-01
We consider the quasi-two-dimensional pseudo-spin-1/2 Kitaev-Heisenberg model proposed for A2IrO3 (A = Li, Na) compounds. The spin-wave excitation spectrum, the sublattice magnetization, and the transition temperatures are calculated in the random phase approximation for four different ordered phases observed in the parameter space of the model: antiferromagnetic, stripe, ferromagnetic, and zigzag phases. The Néel temperature and temperature dependence of the sublattice magnetization are compared with the experimental data on Na2IrO3.
Second order non-linear equations of motion for spinning highly flexible line elements
NASA Technical Reports Server (NTRS)
Salama, M.; Trubert, M.; Essawi, M.; Utku, S.
1982-01-01
The second order nonlinear equations of motion are formulated for spinning line elements having little or no intrinsic structural stiffness. The derivation is based on the extended Hamilton's principle and includes the effect of initial geometric imperfections (axial, curvature, and twist) on the line element dynamics. For comparison with previous work, the nonlinear equations are reduced to a linearized form frequently found in the literature. The comparison revealed several new spin-stiffening terms that have not been previously identified and/or retained. They combine geometric imperfections, rotary inertia, Coriolis, and gyroscopic terms.
ERIC Educational Resources Information Center
Brown, William J.; Vincent, Richard C.
1995-01-01
Analyzes government and print media portrayals of the Reagan administration's policy during Irangate. Finds that the print media continued to fulfill its "watchdog" function by providing critical portrayals of United States policy despite the Reagan administration's attempt to "spin" its own version of Irangate. Examines the Tower Commission…
First-Order Melting of a Weak Spin-Orbit Mott Insulator into a Correlated Metal.
Hogan, Tom; Yamani, Z; Walkup, D; Chen, Xiang; Dally, Rebecca; Ward, Thomas Z; Dean, M P M; Hill, John; Islam, Z; Madhavan, Vidya; Wilson, Stephen D
2015-06-26
The electronic phase diagram of the weak spin-orbit Mott insulator (Sr(1-x)La(x))(3)Ir(2)O(7) is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a narrow regime of nanoscale phase separation comprised of antiferromagnetic, insulating regions and paramagnetic, metallic puddles persisting until x≈0.04. Continued electron doping results in an abrupt, first-order phase boundary where the Néel state is suppressed and a homogenous, correlated, metallic state appears with an enhanced spin susceptibility and local moments. As the metallic state is stabilized, a weak structural distortion develops and suggests a competing instability with the parent spin-orbit Mott state. PMID:26197142
First-order melting of a weak spin-orbit mott insulator into a correlated metal
Hogan, Tom; Yamani, Z.; Walkup, D.; Chen, Xiang; Dally, Rebecca; Ward, Thomas Zac; Dean, M. P. M.; Hill, John P.; Islam, Z.; Madhavan, Vidya; et al
2015-06-25
Herein, the electronic phase diagram of the weak spin-orbit Mott insulator (Sr1-xLax)3Ir2O7 is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a narrow regime of nanoscale phase separation comprised of antiferromagnetic, insulating regions and paramagnetic, metallic puddles persisting until x≈0.04. Continued electron doping results in an abrupt, first-order phase boundary where the Néel state is suppressed and a homogenous, correlated, metallic state appears with an enhanced spin susceptibility and local moments. In conclusion, as the metallic state is stabilized, a weak structural distortion develops and suggests a competingmore » instability with the parent spin-orbit Mott state.« less
First-order melting of a weak spin-orbit mott insulator into a correlated metal
Hogan, Tom; Yamani, Z.; Walkup, D.; Chen, Xiang; Dally, Rebecca; Ward, Thomas Zac; Dean, M. P. M.; Hill, John P.; Islam, Z.; Madhavan, Vidya; Wilson, Stephen D.
2015-06-25
Herein, the electronic phase diagram of the weak spin-orbit Mott insulator (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7} is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a narrow regime of nanoscale phase separation comprised of antiferromagnetic, insulating regions and paramagnetic, metallic puddles persisting until x≈0.04. Continued electron doping results in an abrupt, first-order phase boundary where the Néel state is suppressed and a homogenous, correlated, metallic state appears with an enhanced spin susceptibility and local moments. In conclusion, as the metallic state is stabilized, a weak structural distortion develops and suggests a competing instability with the parent spin-orbit Mott state.
The Search for Magnetic Order in delta-Pu metal using muon spin relaxation
Heffner, R; Ohishi, K; Fluss, M; Morris, G; MacLaughlin, D; Shu, L; Chung, B; McCall, S; Bauer, E; Sarrao, J; Ito, T; Higemoto, W
2006-10-16
We review results from previous muon spin relaxation ({mu}SR) measurements in applied fields of H{sub 0} = 0 and 0.25 T which established an upper limit for the ordered or disordered frozen spin moment above T = 4 K in {delta}-Pu (4.3 at. % Ga) of {micro}{sub ord} {le} 10{sup -3} {mu}{sub B}. In addition, we present new data in H{sub 0} = 0.25 T and 2 T applied field on a highly annealed {delta}-Pu (4.3 at. % Ga) sample. Neither the muon Knight shift (H{sub 0} = 2 T) nor the inhomogeneous linewidths in the new sample show appreciable temperature dependence below about T = 60 K, also consistent with no spin freezing. Recent theoretical arguments advanced to explain these results are mentioned.
First-Order Melting of a Weak Spin-Orbit Mott Insulator into a Correlated Metal
NASA Astrophysics Data System (ADS)
Hogan, Tom; Yamani, Z.; Walkup, D.; Chen, Xiang; Dally, Rebecca; Ward, Thomas Z.; Dean, M. P. M.; Hill, John; Islam, Z.; Madhavan, Vidya; Wilson, Stephen D.
2015-06-01
The electronic phase diagram of the weak spin-orbit Mott insulator (Sr1 -xLax)3Ir2O7 is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a narrow regime of nanoscale phase separation comprised of antiferromagnetic, insulating regions and paramagnetic, metallic puddles persisting until x ≈0.04 . Continued electron doping results in an abrupt, first-order phase boundary where the Néel state is suppressed and a homogenous, correlated, metallic state appears with an enhanced spin susceptibility and local moments. As the metallic state is stabilized, a weak structural distortion develops and suggests a competing instability with the parent spin-orbit Mott state.
Spin-charge order and excitonic effects in sawtooth-like graphene nanoribbons
NASA Astrophysics Data System (ADS)
Wu, Sha; Lu, Wengang; Qi, Jingshan
2016-09-01
In this paper we systematically study electronic structures and excitonic effects in one type of the sawtooth-like graphene nanoribbons. A main feature is that the local magnetism is developed for the certain width and changes with the increase of width. A variety of magnetic orders root in the competition of the short range interaction between the same spin-electrons and long range exchange interaction between opposite spin-electrons. For excitonic effects, the binding energy of degenerate spin-triplets T1 and T-1 is higher than that of T0 for all studied nanoribbons and is size dependent. We reveal the underlying physical mechanism from the charge distributions of excitons and its correlation with the spin-resolved charge density distributions in the ground state. We find that the electrons and holes in degenerate spin-triplets T1 and T-1 are closer together and thus the interaction between them is more strong, while the distribution of electrons and holes is relatively more disperse for T0, indicating the weaker interaction. We hope that these interesting results are able to be detected in the experiment and these multi-performance samples are better utilized in future device applications.
Spin-lattice dynamics simulation of external field effect on magnetic order of ferromagnetic iron
Chui, C. P.; Zhou, Yan
2014-03-15
Modeling of field-induced magnetization in ferromagnetic materials has been an active topic in the last dozen years, yet a dynamic treatment of distance-dependent exchange integral has been lacking. In view of that, we employ spin-lattice dynamics (SLD) simulations to study the external field effect on magnetic order of ferromagnetic iron. Our results show that an external field can increase the inflection point of the temperature. Also the model provides a better description of the effect of spin correlation in response to an external field than the mean-field theory. An external field has a more prominent effect on the long range magnetic order than on the short range counterpart. Furthermore, an external field allows the magnon dispersion curves and the uniform precession modes to exhibit magnetic order variation from their temperature dependence.
NASA Astrophysics Data System (ADS)
Ritter, C.; Ivanov, S. A.; Bazuev, G. V.; Fauth, F.
2016-02-01
The thermal evolution of structural and magnetic details of the orthovanadate TmV O3 , studied in detail by neutron and synchrotron powder diffraction, is reported. Crystallizing in space group Pnma at room temperature, TmV O3 undergoes a first structural phase transition to P 21/a at TOO=180 K , where a G -type orbital ordered state develops. At TS=75 K , a change back to Pnma occurs, and the establishment of C -type orbital order takes place. The V3 + ions order antiferromagnetically with a magnetic propagation vector k =0 below TN 1=105 K , while the T m3 + sublattice orders at TN 2=20 K following the same propagation vector. Between TN 1 and TS, a coexistence of G -type (P 21/a ) and C -type (Pnma) orbital ordered states exists. The P 21/a phase is magnetically separated into two fractions, which adopt a CxCy0 and Gx00 coupling, respectively, while the Pnma volume fraction follows a 0 Gy0 magnetic structure. At TN 2, the appearance of the Tm sublattice magnetization (0 Cy0 ) leads to a spin flop transition of the V sublattice from 0 Gy0 to Gx00 . The results are presented and analyzed in the general context of the series of R V O3 compounds, and they are used to discuss recent magnetization results.
NASA Technical Reports Server (NTRS)
Uemura, Y. J.; Kossler, W. J.; Yu, X. H.; Schone, H. E.; Kempton, J. R.; Stronach, C. E.; Barth, S.; Gygax, F. N.; Hitti, B.; Schenck, A.
1988-01-01
Zero- and longitudinal-field muon spin relaxation measurements on a heavy fermion system CeCu2.1 Si2 have revealed an onset of static magnetic ordering below T(M) approximately 0.8 K, which coexists with superconductivity below T(c) = 0.7 K. The line shapes of the observed muon spin depolarization functions suggest an ordering in either spin glass or incommensurate spin-density-wave state, with a small averaged static moment of the order of 0.1 micro-B per formula unit at T approaches 0.
Mixed-order phase transition in a minimal, diffusion-based spin model
NASA Astrophysics Data System (ADS)
Fronczak, Agata; Fronczak, Piotr
2016-07-01
In this paper we exactly solve, within the grand canonical ensemble, a minimal spin model with the hybrid phase transition. We call the model diffusion based because its Hamiltonian can be recovered from a simple dynamic procedure, which can be seen as an equilibrium statistical mechanics representation of a biased random walk. We outline the derivation of the phase diagram of the model, in which the triple point has the hallmarks of the hybrid transition: discontinuity in the average magnetization and algebraically diverging susceptibilities. At this point, two second-order transition curves meet in equilibrium with the first-order curve, resulting in a prototypical mixed-order behavior.
Mixed-order phase transition in a minimal, diffusion-based spin model.
Fronczak, Agata; Fronczak, Piotr
2016-07-01
In this paper we exactly solve, within the grand canonical ensemble, a minimal spin model with the hybrid phase transition. We call the model diffusion based because its Hamiltonian can be recovered from a simple dynamic procedure, which can be seen as an equilibrium statistical mechanics representation of a biased random walk. We outline the derivation of the phase diagram of the model, in which the triple point has the hallmarks of the hybrid transition: discontinuity in the average magnetization and algebraically diverging susceptibilities. At this point, two second-order transition curves meet in equilibrium with the first-order curve, resulting in a prototypical mixed-order behavior. PMID:27575073
Spin and orbital orderings behind multiferroicity in delafossite and related compounds.
Terada, Noriki
2014-11-12
Coupling between noncollinear magnetic ordering and ferroelectricicty in magnetoelectric multiferroics has been extensively studied in the last decade. Delafossite family compounds with triangular lattice structure provide a great opportunity to study the coupling between spin and electric dipole in multiferroics due to the variety of magnetic phases with different symmetry. This review introduces the magnetic and ferroelectric phase transitions in delafossite ferrites, CuFe(1-x)X(x)O(2) (X = Al, Ga), AgFeO(2) and the related compound α-NaFeO(2). In CuFeO(2), the ferroelectric phase appears under a magnetic field or chemical substitution. The proper screw magnetic ordering with the magnetic point group 21', which has been determined by detailed analysis in neutron diffraction experiments, induces the ferroelectric polarization along the monoclinic b axis in CuFeO2. The cycloidal magnetic orderings are realized in AgFeO(2) and α-NaFeO(2), which are of the point group m1' allowing polarization in the ac plane. The emergence of ferroelectric polarization can be explained by both the extended inverse Dzyaloshinsky-Moriya effect and the d − p hybridization mechanism. These mechanisms are supported by experimental evidence in CuFe(1-x)Ga(x)O2. The polarized neutron diffraction experiment demonstrated one-to-one correspondence between ferroelectric polarization and spin helicity, S(i) × S(j). The incommensurate orbital ordering with 2 Q wave vector, observed by the soft x-ray resonant diffraction experiment, proved that the spin-orbit interaction ties spin and orbital orders to each other, playing a crucial role for the emergence of ferroelectricity in CuFe(1-x)Ga(x)O2. PMID:25336518
Absence of Magnetic Order and Persistent Spin Dynamics in Tb2Ge2O7
NASA Astrophysics Data System (ADS)
Hallas, Alannah; Arevalo-Lopez, Angel; Wilson, Murray; Liu, Lian; Attfield, J. Paul; Uemura, Yasutomo; Wiebe, Chris; Luke, Graeme
2015-03-01
The terbium pyrochlores exhibit many unique magnetic properties, which has generated significant interest in this family of frustrated materials. A candidate spin liquid, Tb2Ti2O7 fails to magnetically order, despite strong antiferromagnetic correlations. The application of external pressure has been found to produce partial antiferromagnetic order in Tb2Ti2O7. Recently, we synthesized a new member of this family, Tb2Ge2O7. Due to the large ionic radii decrease from titanium to germanium, Tb2Ge2O7 can be considered a chemical pressure analog of Tb2Ti2O7. However, neutron scattering measurements revealed an absence of magnetic order in Tb2Ge2O7 down to 20 mK and dominant ferromagnetic correlations. Now, we have investigated the low temperature magnetism of Tb2Ge2O7 with muon spin rotation. Our zero field μSR measurements confirm an absence of static order in Tb2Ge2O7. We find a sharp increase in magnetic correlations below 10 K and persistent spin dynamics down to 25 mK. Our longitudinal field μSR measurements on Tb2Ge2O7 at 25 mK are consistent with a system of fluctuating moments, with a fluctuation rate of 11 MHz. This fluctuation rate is nearly temperature independent below 2.5 K.
43 CFR 3250.13 - What additional BLM orders or instructions govern exploration?
Code of Federal Regulations, 2014 CFR
2014-10-01
... 43 Public Lands: Interior 2 2014-10-01 2014-10-01 false What additional BLM orders or instructions govern exploration? 3250.13 Section 3250.13 Public Lands: Interior Regulations Relating to Public Lands (Continued) BUREAU OF LAND MANAGEMENT, DEPARTMENT OF THE INTERIOR MINERALS MANAGEMENT (3000) GEOTHERMAL RESOURCE LEASING...
48 CFR 252.251-7000 - Ordering from Government supply sources.
Code of Federal Regulations, 2011 CFR
2011-10-01
... 48 Federal Acquisition Regulations System 3 2011-10-01 2011-10-01 false Ordering from Government supply sources. 252.251-7000 Section 252.251-7000 Federal Acquisition Regulations System DEFENSE ACQUISITION REGULATIONS SYSTEM, DEPARTMENT OF DEFENSE CLAUSES AND FORMS SOLICITATION PROVISIONS AND...
Orbital Ordering and Spin-Ladder Formation in La2RuO5
NASA Astrophysics Data System (ADS)
Eyert, V.; Ebbinghaus, S. G.; Kopp, T.
2006-06-01
The semiconductor-semiconductor transition of La2RuO5 is studied by means of augmented spherical wave electronic structure calculations as based on density-functional theory and the local density approximation. This transition has lately been reported to lead to orbital ordering and a quenching of the local spin magnetic moment. Our results hint towards an orbital ordering scenario which, markedly different from the previously proposed scheme, preserves the local S=1 moment at the Ru sites in the low-temperature phase. The unusual magnetic behavior is interpreted by the formation of spin ladders, which result from the structural changes occurring at the transition and are characterized by antiferromagnetic coupling along the rungs.
Second-order Peierls transition in the spin-orbital Kumar-Heisenberg model
NASA Astrophysics Data System (ADS)
Brzezicki, Wojciech; Hagymási, Imre; Dziarmaga, Jacek; Legeza, Örs
2015-05-01
We add a Heisenberg interaction term ∝λ in the one-dimensional SU(2 )⊗XY spin-orbital model introduced by Kumar. At λ =0 the spin and orbital degrees of freedom can be separated by a unitary transformation leading to an exact solution of the model. We show that a finite λ >0 leads to spontaneous dimerization of the system which in the thermodynamic limit becomes a smooth phase transition at λ →0 , whereas it remains discontinuous within the first-order perturbation approach. We present the behavior of the entanglement entropy, energy gap, and dimerization order parameter in the limit of λ →0 confirming the critical behavior. Finally, we show the evidence of another phase transition in the Heisenberg limit, λ →∞ , and give a qualitative analytical explanation of the observed dimerized states both in the limit of small and large λ .
Strong coupling critique of spin fluctuation driven charge order in underdoped cuprates
NASA Astrophysics Data System (ADS)
Mishra, Vivek; Norman, M. R.
2015-08-01
Charge order has emerged as a generic feature of doped cuprates, leading to important questions about its origin and its relation to superconductivity. Recent experiments on two classes of hole doped cuprates indicate a novel d -wave symmetry for the order. These were motivated by earlier spin fluctuation theoretical studies based on an expansion about hot spots in the Brillouin zone that indicated such an order would be competitive with d -wave superconductivity. Here, we reexamine this problem by solving strong coupling equations in the full Brillouin zone for experimentally relevant parameters. We find that bond-oriented order, as seen experimentally, is strongly suppressed. We also include coupling to B1 g phonons and do not see any qualitative change. Our results argue against an itinerant model for the charge order, implying instead that such order is likely due to Coulombic phase separation of the doped holes.
Bordbar, G. H.; Bigdeli, M.
2008-01-15
In this paper, we calculate properties of the spin polarized asymmetrical nuclear matter and neutron star matter, using the lowest order constrained variational (LOCV) method with the AV{sub 18}, Reid93, UV{sub 14}, and AV{sub 14} potentials. According to our results, the spontaneous phase transition to a ferromagnetic state in the asymmetrical nuclear matter as well as neutron star matter do not occur.
ERIC Educational Resources Information Center
Academe, 1989
1989-01-01
Over the last 75 years the AAUP has made progress in specifying its standards of governance and in reconciling traditional governance with collective bargaining. Excerpts from the "Joint Statement on Government of Colleges and Universities" and the "Statement on Academic Government for Institutions Engaged in Collective Bargaining" are presented.…
Probing the antiferromagnetic long-range order with Glauber spin states
NASA Technical Reports Server (NTRS)
Cabrera, Guillermo G.
1994-01-01
It is well known that the ground state of low-dimensional antiferromagnets deviates from Neel states due to strong quantum fluctuations. Even in the presence of long-range order, those fluctuations produce a substantial reduction of the magnetic moment from its saturation value. Numerical simulations in anisotropic antiferromagnetic chains suggest that quantum fluctuations over Neel order appear in the form of localized reversal of pairs of neighboring spins. In this paper, we propose a coherent state representation for the ground state to describe the above situation. In the one-dimensional case, our wave function corresponds to a two-mode Glauber state, when the Neel state is used as a reference, while the boson fields are associated to coherent flip of spin pairs. The coherence manifests itself through the antiferromagnetic long-range order that survives the action of quantum fluctuations. The present representation is different from the standard zero-point spin wave state, and is asymptotically exact in the limit of strong anisotropy. The fermionic version of the theory, obtained through the Jordan-Wigner transformation, is also investigated.
NASA Astrophysics Data System (ADS)
Huang, Cheng-Yi; Tsai, Wei-Feng; Wang, Yung Jui; Lin, Hsin; Bansil, Arun
2014-03-01
We discuss spin reorientation phenomena, which may or may not yield gap formation, on the surface of topological crystalline insulators Pb1-xSnx(Te, Se) under various applied strains. The low-energy surface electrons on the (001) surface behave like massless Dirac particles with four Dirac points centered along the intersection of the mirror (xz or yz) plane and the surface plane. We use a four-band k.p model, which captures the spin and orbital texture of the surface states around surface X (or Y) point up to the energy around the Lifshitz transition, and systematically study effects of the applied strain. In contrast to the case without any strain, where the absence of the out-of-the-plane spin component is guaranteed by both the mirror and the time-reversal symmetries, we find that without time-reversal symmetry breaking, the hedgehog-like spin textures associated with a gap formation can be induced by the strain only, breaking the xz mirror symmetry. The other cases cannot induce a gap at Dirac points. We also investigate interaction-driven competing orders under the strain and obtain a phase diagram at the mean-field level to reveal the possible novel surface states in the system.
Spin exciton formation inside the hidden order phase of CeB6.
Akbari, Alireza; Thalmeier, Peter
2012-04-01
The heavy fermion metal CeB(6) exhibits a hidden order of the antiferroquadrupolar (AFQ) type below T(Q)=3.2 K and a subsequent antiferromagnetic (AFM) order at T(N)=2.3 K. It was interpreted as an ordering of the quadrupole and dipole moments of a Γ(8) quartet of localized Ce 4f(1) electrons. This established picture has been profoundly shaken by recent inelastic neutron scattering (G. Friemel et al., arXiv:1111.4151) that found the evolution of a feedback spin exciton resonance within the hidden order phase at the AFQ wave vector which is stabilized by the AFM order. We develop an alternative theory based on a fourfold degenerate Anderson lattice model, including both order parameters as particle-hole condensates of itinerant heavy quasiparticles. This explains in a natural way the appearance of the spin exciton resonance and the momentum dependence of its spectral weight, in particular, around the AFQ vector and its rapid disappearance in the disordered phase. Analogies to the feedback effect in unconventional heavy fermion superconductors are pointed out. PMID:22540812
Suppression of charge and spin order in confined NdNiO3 layers
NASA Astrophysics Data System (ADS)
Disa, Ankit; Kumah, Divine; Malashevich, Andrei; Ismail-Beigi, Sohrab; Walker, Fred; Ahn, Charles
Atomic-layer synthesis allows one to study and control the complex phase behavior correlated systems by controllably modifying dimensionality and interfacial constraints. To this end, the rare-earth nickelates (RNiO3) embody a remarkable model system, as exhibited by the bulk metal-insulator and paramagnetic-antiferromagnetic ordering transitions, which are sensitive to structural and electronic conditions. We present evidence from transport, x-ray absorption, and resonant x-ray scattering measurements of NdNiO3/NdAlO3 superlattices of a suppression of charge and spin order induced by interfacial confinement. We find that the spectroscopic signatures of charge localization and antiferromagnetic ordering remain for NdNiO3 layers thicker than a single unit cell. The disappearance of ground state order in single NdNiO3 layers is attributed to enhanced eg orbital polarization from the interaction with the NdAlO3 confining layers. We also observe a crossover region of thickness with no metal-insulator transition but distinct charge and spin ordering temperatures. These findings shed light on the interplay between competing ground states in nickelates and help guide efforts to controlling long-range order in such systems.
A Self-Averaging ``Order Parameter'' for the Sherrington-Kirkpatrick Spin Glass Model
NASA Astrophysics Data System (ADS)
Wreszinski, Walter F.; Bolina, Oscar
2004-09-01
Following an idea of van Enter and Griffiths, we define a self-averaging parameter for the Sherrington-Kirkpatrick (SK) spin glass which is a self-averaging version of the order parameter introduced by Aizenman, Lebowitz and Ruelle. It is strictly positive at low temperature and zero at sufficiently high temperature. The proof is based on the recent construction of the thermodynamic limit of the free energy by Guerra and Toninelli. We also discuss how our definition compares with various existing definitions of order-parameter like quantities.
Magnetic Order in the Mixed-Spin Triangular Lattice Antiferromagnet NaxMnO2
NASA Astrophysics Data System (ADS)
Chisnell, Robin; Parshall, Dan; Li, Xin; Larson, Amber; Suzuki, Takehito; Checkelsky, Joseph; Rodriguez, Efrain; Lynn, Jeffrey
NaxTMO2 (TM = transition metal) materials consist of alternating layers of Na and TM ions with the TM ions arranged on a geometrically frustrated triangular lattice. Na can be easily and reversibly removed from these materials, making them of interest for application in rechargeable batteries and allowing for exploration of their rich phase diagrams as a function of Na concentration. Na ordering is an important factor in ground state selection, and is driven by electrostatic interactions in many NaxTMO2 systems. The TM = Mn series differs in that Na ordering is driven by a cooperative Jahn-Teller effect, due to the coexistence of Jahn-Teller active Mn3+ and inactive Mn4+ ions. This effect also results in an ordered arrangement of the Mn3+ and Mn4+ ions, and thus of spin-2 and spin-3/2 moments. For x = 5/8, we have recently shown the coexistence of charge and magnetic stripe orderings. Here, we present the results of neutron diffraction measurements performed on single crystal samples of NaxMnO2 and discuss the details of the magnetic structure in the magnetically ordered phase.
Spin and orbital ordering in Y1-xLaxVO₃
Yan, J.-Q.; Zhou, J.-S.; Cheng, J. G.; Goodenough, J. B.; Ren, Y.; Llobet, A.; McQueeney, R. J.
2011-12-02
The spin and orbital ordering in Y1-xLaxVO₃ (0.30 ≤ x ≤ 1.0) has been studied to map out the phase diagram over the whole doping range 0 ≤ x ≤ 1. The phase diagram is compared with that for RVO₃ (R = rare earth or Y) perovskites without A-site variance. For x > 0.20, no long-range orbital ordering was observed above the magnetic ordering temperature TN; the magnetic order is accompanied by a lattice anomaly at a Tt ≤ TN as in LaVO₃. The magnetic ordering below Tt ≤ TN is G type in the compositional range 0.20 ≤ xmore » ≤ 0.40 and C type in the range 0.738 ≤ x ≤ 1.0. Magnetization and neutron powder diffraction measurements point to the coexistence below TN of the two magnetic phases in the compositional range 0.4 < x < 0.738. Samples in the compositional range 0.20 < x ≤ 1.0 are characterized by an additional suppression of a glasslike thermal conductivity in the temperature interval TN < T < T* and a change in the slope of 1/χ(T). We argue that T* represents a temperature below which spin and orbital fluctuations couple together via λL∙S.« less
Thermalization, Charge Ordering, and other Recent Developments in Artificial Spin Ice
NASA Astrophysics Data System (ADS)
Schiffer, Peter
2015-03-01
Artificial spin ice consists of arrays of lithographically fabricated single-domain ferromagnetic elements, arranged in different geometries such that the magnetostatic interactions between the moments are frustrated. Magnetic force microscopy imaging of these arrays allows us to study the accommodation of frustration through the local correlations between the moments as a function of both the strength of the interactions and the geometry of the frustration. The interactions can be closely mapped onto those of the ``spin ice'' materials, and allow a detailed analysis of the local correlations and monopole-like excitations. We have probed a number of different lattice geometries and find both local ordering and disordered states that match classic models for frustrated spin systems. Our recent work has focused on thermalization of these arrays as well as investigation of lattice geometries that are unavailable in natural systems and are specifically designed to exhibit unusual behavior associated with frustration, e.g., the shakti lattice. Thermalization reveals ordering both of the moments and of the effective magnetic charges that characterize correlated many-body dynamics in these systems. Other recent work has involved studies of return point memory as well as measurements of electrical transport in these systems. This work was primarily funded by the US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division under Grant No. DE-SC0010778.
Guo, Y. M.; Ruan, M. Y.; Cheng, J. J.; Sun, Y. C.; Ouyang, Z. W. Xia, Z. C.; Rao, G. H.
2015-06-14
High-field electron spin resonance (ESR) has been employed to study the antiferromagnetic (AFM) ordering state (T < T{sub N} = 55 K) of spin-chain multiferroic Gd{sub 2}BaNiO{sub 5}. The spin reorientation at T{sub SR} = 24 K is well characterized by the temperature-dependent ESR spectra. The magnetization data evidence a field-induced spin-flop transition at 2 K. The frequency-field relationship of the ESR data can be explained by conventional AFM resonance theory with uniaxial anisotropy, in good agreement with magnetization data. Related discussion on zero-field spin gap is presented.
Spin Ferroquadrupolar Order in the Nematic Phase of FeSe
NASA Astrophysics Data System (ADS)
Wang, Zhentao; Hu, Wen-Jun; Nevidomskyy, Andriy H.
2016-06-01
We provide evidence that spin ferroquadrupolar (FQ) order is the likely ground state in the nonmagnetic nematic phase of stoichiometric FeSe. By studying the variational mean-field phase diagram of a bilinear-biquadratic Heisenberg model up to the 2nd nearest neighbor, we find the FQ phase in close proximity to the columnar antiferromagnet commonly realized in iron-based superconductors; the stability of the FQ phase is further verified by the density matrix renormalization group. The dynamical spin structure factor in the FQ state is calculated with flavor-wave theory, which yields a qualitatively consistent result with inelastic neutron scattering experiments on FeSe at both low and high energies. We verify that FQ can coexist with C4 breaking environments in the mean-field calculation, and further discuss the possibility that quantum fluctuations in FQ act as a source of nematicity.
Spin Ferroquadrupolar Order in the Nematic Phase of FeSe.
Wang, Zhentao; Hu, Wen-Jun; Nevidomskyy, Andriy H
2016-06-17
We provide evidence that spin ferroquadrupolar (FQ) order is the likely ground state in the nonmagnetic nematic phase of stoichiometric FeSe. By studying the variational mean-field phase diagram of a bilinear-biquadratic Heisenberg model up to the 2nd nearest neighbor, we find the FQ phase in close proximity to the columnar antiferromagnet commonly realized in iron-based superconductors; the stability of the FQ phase is further verified by the density matrix renormalization group. The dynamical spin structure factor in the FQ state is calculated with flavor-wave theory, which yields a qualitatively consistent result with inelastic neutron scattering experiments on FeSe at both low and high energies. We verify that FQ can coexist with C_{4} breaking environments in the mean-field calculation, and further discuss the possibility that quantum fluctuations in FQ act as a source of nematicity. PMID:27367404
Confinement transition to density wave order in metallic doped spin liquids
NASA Astrophysics Data System (ADS)
Patel, Aavishkar A.; Chowdhury, Debanjan; Allais, Andrea; Sachdev, Subir
2016-04-01
Insulating quantum spin liquids can undergo a confinement transition to a valence bond solid via the condensation of topological excitations of the associated gauge theory. We extend the theory of such transitions to fractionalized Fermi liquids (FL*): These are metallic doped spin liquids in which the Fermi surfaces only have gauge neutral quasiparticles. Using insights from a duality transform on a doped quantum dimer model for the U(1)-FL* state, we show that projective symmetry group of the theory of the topological excitations remains unmodified, but the Fermi surfaces can lead to additional frustrating interactions. We propose a theory for the confinement transition of Z2-FL* states via the condensation of visons. A variety of confining, incommensurate density wave states are possible, including some that are similar to the incommensurate d -form factor density wave order observed in several recent experiments on the cuprate superconductors.
Thermodynamic studies at the charge-ordering and spin-Peierls transitions in (TMTTF)2X
NASA Astrophysics Data System (ADS)
de Souza, Mariano; Brühl, Andreas; Müller, Jens; Foury-Leylekian, Pascale; Moradpour, Alec; Pouget, Jean-Paul; Lang, Michael
2009-03-01
We report results of high-resolution thermal expansion measurements on the charge-ordering (TCO) and spin-Peierls (TSP) transition in (TMTTF)2X for X=AsF6 and PF6. Based on distinct lattice effects observed at TCO in the c*-axis expansivity, a scheme is proposed which involves a charge modulation along the TMTTF stacks and its coupling to displacements of the anions. It is also the c*-axis expansivity which is most strongly affected by the transition at TSP. The combination of expansivity and specific heat results for the X=AsF6 salt enables us to separate for both quantities the contribution associated with the spin-Peierls transition from the ordinary lattice effects and to provide a thermodynamic determination of the uniaxial-pressure dependence of TSP.
Analytical high-order post-Newtonian expansions for spinning extreme mass ratio binaries
NASA Astrophysics Data System (ADS)
Kavanagh, Chris; Ottewill, Adrian C.; Wardell, Barry
2016-06-01
We present an analytic computation of Detweiler's redshift invariant for a point mass in a circular orbit around a Kerr black hole, giving results up to 8.5 post-Newtonian order while making no assumptions on the magnitude of the spin of the black hole. Our calculation is based on the functional series method of Mano, Suzuki and Takasugi, and employs a rigorous mode-sum regularization prescription based on the Detweiler-Whiting singular-regular decomposition. The approximations used in our approach are minimal; we use the standard self-force expansion to linear order in the mass ratio, and the standard post-Newtonian expansion in the separation of the binary. A key advantage of this approach is that it produces expressions that include contributions at all orders in the spin of the Kerr black hole. While this work applies the method to the specific case of Detweiler's redshift invariant, it can be readily extended to other gauge-invariant quantities and to higher post-Newtonian orders.
Effect of random field disorder on the first order transition in p-spin interaction model
NASA Astrophysics Data System (ADS)
Sumedha; Singh, Sushant K.
2016-01-01
We study the random field p-spin model with Ising spins on a fully connected graph using the theory of large deviations in this paper. This is a good model to study the effect of quenched random field on systems which have a sharp first order transition in the pure state. For p = 2, the phase-diagram of the model, for bimodal distribution of the random field, has been well studied and is known to undergo a continuous transition for lower values of the random field (h) and a first order transition beyond a threshold, htp(≈ 0.439) . We find the phase diagram of the model, for all p ≥ 2, with bimodal random field distribution, using large deviation techniques. We also look at the fluctuations in the system by calculating the magnetic susceptibility. For p = 2, beyond the tricritical point in the regime of first order transition, we find that for htp < h < 0.447, magnetic susceptibility increases rapidly (even though it never diverges) as one approaches the transition from the high temperature side. On the other hand, for 0.447 < h ≤ 0.5, the high temperature behaviour is well described by the Curie-Weiss law. For all p ≥ 2, we find that for larger magnitudes of the random field (h >ho = 1 / p!), the system does not show ferromagnetic order even at zero temperature. We find that the magnetic susceptibility for p ≥ 3 is discontinuous at the transition point for h
NASA Astrophysics Data System (ADS)
Negi, D. S.; Loukya, B.; Datta, R.
2015-12-01
We report on the observation of Co vacancy (VCo) induced charge ordering and ferromagnetism in CoO epitaxial thin film. The ordering is associated with the coexistence of commensurate, incommensurate, and discommensurate electronic phases. Density functional theory calculation indicates the origin of ordering in Co atoms undergoing high spin to low spin transition immediately surrounding the VCo(16.6 at. %). Electron magnetic chiral dichroism experiment confirms the ferromagnetic signal at uncompensated Co spins. Such a native defects induced coexistence of different electronic phases at room temperature in a simple compound CoO is unique and adds to the richness of the field with the possibility of practical device application.
NASA Astrophysics Data System (ADS)
Gong, Shoushu; Zhu, Wei; Balents, Leon; Sheng, Dongning
2015-03-01
We studied the extended spin- 1 / 2 kagome model with the first neighbor (J1), the second (J2) and third neighbor (J3) couplings using density matrix renormalization group. We established a quantum phase diagram for 0 <= J 2 <= 0 . 25J1 and 0 <=J3 <=J1 , where we find a q = (0 , 0) Neel phase, a chiral spin liquid (CSL), a cuboc1 phase that breaks both time-reversal and spin rotational symmetries, and a valence-bond solid at the neighbor of the Heisenberg model, where a possible Z2 spin liquid has been previously identified. Interestingly, the classical cuboc1 phase could survive in the spin- 1 / 2 system with strong quantum fluctuations, and the CSL emerges between the q = (0 , 0) and the cuboc1 phases. We discover that the CSL has the short spin correlation pattern consistent with the cuboc1 phase, but the chiral order structure is totally different. The CSL might be understood as a result of the competitions between the q = (0 , 0) and the cuboc1 phases in the presence of strong quantum fluctuations. We further studied the quantum phase transitions from the CSL to the magnetically ordered phases, and to the possible Z2 spin liquid of the Heisenberg kagome model. Interestingly, the exotic continuous topological phase transition might be realized in the system.
Porto, Rafael A.; Ross, Andreas; Rothstein, Ira Z. E-mail: andreasr@andrew.cmu.edu
2012-09-01
Using the NRGR effective field theory formalism we calculate the remaining source multipole moments necessary to obtain the spin contributions to the gravitational wave amplitude to 2.5 Post-Newtonian (PN) order. We also reproduce the tail contribution to the waveform linear in spin at 2.5PN arising from the nonlinear interaction between the current quadrupole and the mass monopole.
NASA Astrophysics Data System (ADS)
Sarkar, Tapati; Ivanov, Sergey A.; Bazuev, G. V.; Nordblad, Per; Mathieu, Roland
2016-07-01
Synthesis, crystal structure and magnetization measurements of phase pure polycrystalline RVO3 (R=Lu, Yb and Tm) are reported. The compounds were stabilized in the orthorhombic structure by thermal treatment of the respective precursors (RVO4) in a reducing atmosphere. Special pressure treatment was carried out during the synthesis to ensure phase pure samples without secondary phases. Magnetization measurements reveal the presence of two spin ordering temperatures in the samples. Interestingly, at the lower spin ordering temperature, TSO2, the uncompensated excess moment of the antiferromagnetic spin structure has different field dependences above and below TSO2, causing a jump in the thermal evolution of the magnetization that changes sign with increasing field strength. This jump is associated with the reported magnetic and orbital rearrangement in the samples, and the different spin configurations in the C- and G-type antiferromagnetic structures.
Pulsed NMR in the nuclear spin ordered phases of solid 3He in a silver sinter
NASA Astrophysics Data System (ADS)
Millan-Chacartegui, Carmen; Schuberth, Erwin A.; Deppe, Frank; Schöttl, Stephan
2003-05-01
To obtain the exact spin structure of the nuclear magnetically ordered phases of solid 3He, in the BCC lattice called U2D2 and high field phase, both occurring below about 1 mK, we started a project of neutron scattering from the solid at the Hahn-Meitner Institut, Berlin. This experiment faces three main difficulties: to cool the solid to temperatures below 1 mK (or even much lower in the case of the HCP lattice), to keep it there under neutron flux, and to grow a single crystal within the sintered material needed for this purpose. As a first step we have performed pulsed NMR measurements in the ordered phases of solid 3He in a silver sinter of 700 Å particle size down to temperatures of 600 μK at various molar volumes. The samples remained in the ordered state for as long as 110 h.
Long-range order for the spin-1 Heisenberg model with a small antiferromagnetic interaction
Lees, Benjamin
2014-09-15
We look at the general SU(2) invariant spin-1 Heisenberg model. This family includes the well-known Heisenberg ferromagnet and antiferromagnet as well as the interesting nematic (biquadratic) and the largely mysterious staggered-nematic interaction. Long range order is proved using the method of reflection positivity and infrared bounds on a purely nematic interaction. This is achieved through the use of a type of matrix representation of the interaction making clear several identities that would not otherwise be noticed. Using the reflection positivity of the antiferromagnetic interaction one can then show that the result is maintained if we also include an antiferromagnetic interaction that is sufficiently small.
NASA Astrophysics Data System (ADS)
Günther, Stefan; Spezzani, Carlo; Ciprian, Roberta; Grazioli, Cesare; Ressel, Barbara; Coreno, Marcello; Poletto, Luca; Miotti, Paolo; Sacchi, Maurizio; Panaccione, Giancarlo; Uhlíř, Vojtěch; Fullerton, Eric E.; De Ninno, Giovanni; Back, Christian H.
2014-11-01
We use element-resolved IR-pump/extreme ultraviolet-probe experiments to disentangle the ultrafast interplay of the magnetic sublattices of an ordered crystalline magnetic alloy. As a paradigmatic example, we investigate the case of the FeRh alloy, which shows a delayed response for the different components. Furthermore, a detailed time-resolved magneto-optic study shows that the data can be analyzed by only assuming Elliot-Yafet-like scattering, as the underlying mechanism for ultrafast demagnetization, resulting in an unexpected nonmonotonic dependence of the spin-flip rate, as a function of quenching.
Magnetic order and spin-flop transitions in the cobalt-doped multiferroic Mn1-xCoxWO4
NASA Astrophysics Data System (ADS)
Ye, Feng; Chi, Songxue; Fernandez-Baca, Jaime A.; Cao, Huibo; Liang, K.-C.; Wang, Yaqi; Lorenz, Bernd; Chu, C. W.
2012-09-01
We present a comprehensive single-crystal neutron diffraction investigation of the Mn1-xCoxWO4 with 0.02≤x≤0.30. At lower concentration x≤0.05, the system is quickly driven into the multiferroic phase with spin structure forming an elliptical spiral order similar to the parent compound. The reduction of electric polarization is ascribed to the tilting of the spiral plane. For x˜0.075, the magnetic structure undergoes a spin-flop transition that is characterized by a sudden rotation of the spin helix envelope into the ac plane. This spin structure persists for concentration up to x=0.15, where additional competing magnetic orders appear at low temperature. For 0.17≤x≤0.30, the system experiences another spin-flop transition and recovers the low-x spiral spin configuration. A simple commensurate spin structure with q⃗=(0.5,0,0) is found to coexist with the incommensurate spiral order. The complex evolution of magnetic structure in Co doped MnWO4 contrasts sharply with other transition metal ion doped Mn1-xAxWO4 (A=Zn, Mg, Fe) where the chemical substitutions stabilize only one type of magnetic structure. The rich phase diagram of Mn1-xCoxWO4 results from the interplay between magnetic frustration and spin anisotropy of the Co ions.
Murata, Ken-ichiro; Tanaka, Hajime
2015-01-01
A liquid–liquid transition (LLT) in a single-component substance is an unconventional phase transition from one liquid to another. LLT has recently attracted considerable attention because of its fundamental importance in our understanding of the liquid state. To access the order parameter governing LLT from a microscopic viewpoint, here we follow the structural evolution during the LLT of an organic molecular liquid, triphenyl phosphite (TPP), by time-resolved small- and wide-angle X-ray scattering measurements. We find that locally favored clusters, whose characteristic size is a few nanometers, are spontaneously formed and their number density monotonically increases during LLT. This strongly suggests that the order parameter of LLT is the number density of locally favored structures and of nonconserved nature. We also show that the locally favored structures are distinct from the crystal structure and these two types of orderings compete with each other. Thus, our study not only experimentally identifies the structural order parameter governing LLT, but also may settle a long-standing debate on the nature of the transition in TPP, i.e., whether the transition is LLT or merely microcrystal formation. PMID:25918385
NASA Astrophysics Data System (ADS)
Tatton, Andrew S.; Frantsuzov, Ilya; Brown, Steven P.; Hodgkinson, Paul
2012-02-01
We recently noted [R. K. Harris, P. Hodgkinson, V. Zorin, J.-N. Dumez, B. Elena, L. Emsley, E. Salager, and R. Stein, Magn. Reson. Chem. 48, S103 (2010), 10.1002/mrc.2636] anomalous shifts in apparent 1H chemical shifts in experiments using 1H homonuclear decoupling sequences to acquire high-resolution 1H NMR spectra for organic solids under magic-angle spinning (MAS). Analogous effects were also observed in numerical simulations of model 13C,1H spin systems under homonuclear decoupling and involving large 13C,1H dipolar couplings. While the heteronuclear coupling is generally assumed to be efficiently suppressed by sample spinning at the magic angle, we show that under conditions typically used in solid-state NMR, there is a significant third-order cross-term from this coupling under the conditions of simultaneous MAS and homonuclear decoupling for spins directly bonded to 1H. This term, which is of the order of 100 Hz under typical conditions, explains the anomalous behaviour observed on both 1H and 13C spins, including the fast dephasing observed in 13C{1H} heteronuclear spin-echo experiments under 1H homonuclear decoupling. Strategies for minimising the impact of this effect are also discussed.
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2010-10-01
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Microviscosity of human erythrocytes studied using hypophosphite two-spin order relaxation.
Price, W S; Perng, B C; Tsai, C L; Hwang, L P
1992-01-01
A new 31P NMR method is used to probe the cytoplasmic viscosity of human erythrocytes. The method is based on observing two-spin order relaxation of the 31P atom of the hypophosphite ion. This method is superior to our previous method, using the longitudinal relaxation time of the ion, because random field effects such as intermolecular dipole-dipole relaxation can be separated from intramolecular relaxation. This allows a more accurate determination of the effective reorientational correlation time from the measured intramolecular relaxation because it is now unaffected by random field effects. The new method also provides a means by which to estimate the random field effects. Both two-spin order and proton-decoupled T1 measurements were conducted on hypophosphite in water solutions at various temperatures, glycerol solutions of various viscosities, and in erythrocyte samples of various cell volumes. The results show that the effective reorientational correlation time of the hypophosphite ion varies from 7.2 to 15.2 ps in the cytoplasm of cells ranging in volume from 102 to 56 fl cells. PMID:1504239
Spin excitations in a model of FeSe with orbital ordering
NASA Astrophysics Data System (ADS)
Kreisel, A.; Mukherjee, Shantanu; Hirschfeld, P. J.; Andersen, Brian M.
2015-12-01
We present a theoretical study of the dynamical spin susceptibility for the intriguing Fe-based superconductor FeSe, based on a tight-binding model developed to account for the temperature-dependent band structure in this system. The model allows for orbital ordering in the dx z/dy z channel below the structural transition and presents a strongly C4-symmetry-broken Fermi surface at low temperatures which accounts for the nematic properties of this material. The calculated spin excitations are peaked at wave vector (π ,0 ) in the 1-Fe Brillouin zone, with a broad maximum at energies of order a few meV. In this range, the occurrence of superconductivity sharpens this peak in energy, creating a (π ,0 ) "neutron resonance" as seen in recent experiments. With the exception of the quite low energy scale of these fluctuations, these results are roughly similar to standard behavior in Fe pnictide systems. At higher energies, however, intensity increases and shifts to wave vectors along the (π ,0 )-(π ,π ) line. We compare with existing inelastic neutron experiments and NMR data, and give predictions for further studies.
Nematic and spin-charge orders driven by hole-doping a charge-transfer insulator
NASA Astrophysics Data System (ADS)
Fischer, Mark H.; Wu, Si; Lawler, Michael; Paramekanti, Arun; Kim, Eun-Ah
2014-09-01
Recent experimental discoveries have brought a diverse set of broken symmetry states to the center stage of research on cuprate superconductors. Here, we focus on a thematic understanding of the diverse phenomenology by exploring a strong-coupling mechanism of symmetry breaking driven by frustration of antiferromagnetic (AFM) order. We achieve this through a variational study of a three-band model of the CuO2 plane with Kondo type exchange couplings between doped oxygen holes and classical copper spins. Two main findings from this strong-coupling multi-band perspective are (1) that the symmetry hierarchy of spin stripe, charge stripe, intra-unit-cell nematic order and isotropic phases are all accessible microscopically within the model, (2) many symmetry-breaking patterns compete with energy differences within a few meV per Cu atom to produce a rich phase diagram. These results indicate that the diverse phenomenology of broken-symmetry states in hole-doped AFM charge-transfer insulators may indeed arise from hole-doped frustration of antiferromagnetism.
Spin state ordering of strongly correlating LaCoO3 induced at ultrahigh magnetic fields
NASA Astrophysics Data System (ADS)
Ikeda, Akihiko; Nomura, Toshihiro; Matsuda, Yasuhiro H.; Matsuo, Akira; Kindo, Koichi; Sato, Keisuke
2016-06-01
Magnetization measurements of LaCoO3 have been carried out up to 133 T, generated with a destructive pulse magnet at a wide temperature range from 2 to 120 K. A novel magnetic transition was found at B >100 T and T >T*=32 ±5 K, which is characterized by its transition field increasing with increasing temperature. At T
Vestigial nematicity from spin and/or charge order in the cuprates
NASA Astrophysics Data System (ADS)
Nie, Laimei; Maharaj, Akash; Fradkin, Eduardo; Kivelson, Steven
Nematic order (C4 rotation symmetry breaking) has manifested itself in a variety of materials in the cuprates family, yet its origin remains debatable, with possible links to lattice, charge, and spin degrees of freedom across different doping regimes. We propose an effective field theory of a layered system with incommensurate, intertwined spin- and charge-density wave (SDW and CDW) orders, each of which consists of two components related by C4 rotations. Using a variational free energy approach, we study the growth of the associated nematicity from partially melting those density waves by either increasing temperature or adding quenched disorder. Under the assumption that the zero-disorder, zero-interaction SDW transition temperature is higher than CDW at small doping (and vice versa for large doping), we find that for the general case with finite disorder and interactions there is a universal nematic transition across the entire doping range, accompanied by SDW and CDW transitions (or strong fluctuations at large enough disorder) at lower temperatures. We also discuss the issues concerning the difference between La-based materials and the other hole-doped cuprates.
Second order formalism for spin (1/2) fermions and Compton scattering
Delgado-Acosta, E. G.; Napsuciale, Mauro; Rodriguez, Simon
2011-04-01
We develop a second order formalism for massive spin 1/2 fermions based on the projection over Poincare invariant subspaces in the ((1/2),0)+(0,(1/2)) representation of the homogeneous Lorentz group. Using the U(1){sub em} gauge principle we obtain a second order description for the electromagnetic interactions of a spin 1/2 fermion with two free parameters, the gyromagnetic factor g and a parameter {xi} related to odd-parity Lorentz structures. We calculate Compton scattering in this formalism. In the particular case g=2, {xi}=0, and for states with well-defined parity, we recover Dirac results. In general, we find the correct classical limit and a finite value r{sub c}{sup 2} for the forward differential cross section, independent of the photon energy and of the value of the parameters g and {xi}. The differential cross section vanishes at high energies for all g, {xi} except in the forward direction. The total cross section at high energies vanishes only for g=2, {xi}=0. We argue that this formalism is more convenient than Dirac theory in the description of low energy electromagnetic properties of baryons and illustrate the point with the proton case.
Ge, Mingtao; Freed, Jack H.
2009-01-01
Abstract A spin-labeling study of interactions of a fusion peptide from the hemagglutinin of the influenza virus, wt20, and a fusion-inactive mutant ΔG1 with dimyristoylphosphatidylcholine (DMPC) and 1-palmitoyl-2-oleoyl-phosphatdylcholine bilayers was performed. We found that upon binding of wt20, the ordering of headgroups and the ordering of acyl chains near the headgroup increased significantly, in a manner consistent with a cooperative phenomenon. However, changes in the order at the end of the acyl chains were negligible. The ordering effect of wt20 on the headgroup was much stronger at pH 5 than at pH 7. No effect of ΔG1 binding on the order of bilayers was evident. We also found that 1-palmitoyl-2-hydroxyl phosphatidylcholine, a membrane-fusion inhibitor, decreased the ordering of DMPC headgroups, whereas arachidonic acid, a membrane-fusion promoter, increased the ordering of DMPC headgroups. These results suggest that increases in headgroup ordering may be important for membrane fusion. We propose that upon binding of wt20, which is known to affect only the outer leaflet of the bilayer, this outer leaflet becomes more ordered, and thus more solid-like. Then the coupling between the hardened outer leaflet and the softer inner leaflet generates bending stresses in the bilayer, which tend to increase the negative curvature of the bilayer. We suggest that the increased ordering in the headgroup region enhances dipolar interactions and lowers electrostatic energy, which may provide an energy source for membrane fusion. Possible roles of bending stresses in promoting membrane fusion are discussed. PMID:19527651
Ferroic ordering and charge-spin-lattice order coupling in Gd doped Fe3O4 nanoparticles
NASA Astrophysics Data System (ADS)
Laha, Suvra; Abdelhamid, Ehab; Palihawadana Arachchige, Maheshika; Dixit, Ambesh; Lawes, Gavin; Naik, Vaman; Naik, Ratna
Rare earth doped spinels have been extensively studied for their potential applications in magneto-optical recording and as MRI contrast agents. In the present study, we have investigated the effect of gadolinium doping (1-5 at.%) on the magnetic and dielectric properties of Fe3O4nanoparticles synthesized by the chemical co-precipitation method. The structure and morphology of the as-synthesized gadolinium doped Fe3O4(Gd-Fe3O4) nanoparticles were characterized by XRD, SEM and TEM, and the magnetic properties were measured by a Quantum Design physical property measurement system. We find that the penetration of excess Gd3+ ions into Fe3O4 spinel matrix significantly influences the average crystallite size and saturation magnetization in Gd-Fe3O4. The average crystallite size, estimated from XRD using Scherrer equation, increases with increasing Gd doping percentage and the saturation magnetization drops monotonically with excess Gd3+ ions. Interestingly, Gd- Fe3O4develops enhanced ferroelectric ordering at low temperatures. The details of the temperature dependent dielectric, ferroelectric and magnetocapacitance measurements to understand the onset of charge-spin-lattice coupling in Gd-Fe3O4 system will be presented.
An alternative order-parameter for non-equilibrium generalized spin models on honeycomb lattices
NASA Astrophysics Data System (ADS)
Sastre, Francisco; Henkel, Malte
2016-04-01
An alternative definition for the order-parameter is proposed, for a family of non-equilibrium spin models with up-down symmetry on honeycomb lattices, and which depends on two parameters. In contrast to the usual definition, our proposal takes into account that each site of the lattice can be associated with a local temperature which depends on the local environment of each site. Using the generalised voter motel as a test case, we analyse the phase diagram and the critical exponents in the stationary state and compare the results of the standard order-parameter with the ones following from our new proposal, on the honeycomb lattice. The stationary phase transition is in the Ising universality class. Finite-size corrections are also studied and the Wegner exponent is estimated as ω =1.06(9).
Spin polarized photons from an axially charged plasma at weak coupling: Complete leading order
NASA Astrophysics Data System (ADS)
Mamo, Kiminad A.; Yee, Ho-Ung
2016-03-01
In the presence of (approximately conserved) axial charge in the QCD plasma at finite temperature, the emitted photons are spin aligned, which is a unique P - and C P -odd signature of axial charge in the photon emission observables. We compute this "P -odd photon emission rate" in a weak coupling regime at a high temperature limit to complete leading order in the QCD coupling constant: the leading log as well as the constant under the log. As in the P -even total emission rate in the literature, the computation of the P -odd emission rate at leading order consists of three parts: (1) Compton and pair annihilation processes with hard momentum exchange, (2) soft t - and u -channel contributions with hard thermal loop resummation, (3) Landau-Pomeranchuk-Migdal resummation of collinear bremsstrahlung and pair annihilation. We present analytical and numerical evaluations of these contributions to our P -odd photon emission rate observable.
First-Order Transition in a Spin Model for Self-Organization
NASA Astrophysics Data System (ADS)
Bauvin, R.; Kamp, Y.
The paper examines the emergence of self-organization in a population where tandem recruitment is combined with individual memory. The time evolution is modeled as a two-dimensional spin system with local interaction along the time axis and a mean-field interaction along the other axis. We generalize a previous result obtained with this model from the case of two sources to the multisource situation and show a twofold connection with the Potts model. First, when individual memory exceeds a critical value, a phase transition sets in, which is second order for two sources but first order beyond, similarly to the mean-field theory of the Potts model. In addition, the self-organization problem considered here relies on a special case of the one-dimensional nearest-neighbor Potts model with external field, which is shown to be explicitly solvable.
Magnetic ordering in tetragonal FeS: Evidence for strong itinerant spin fluctuations
Kwon, K.D.; Refson, K.; Bone, S.; Qiao, R.; Yang, W.; Liu, Z.; Sposito, G.
2010-11-01
Mackinawite is a naturally occurring layer-type FeS mineral important in biogeochemical cycles and, more recently, in the development of microbial fuel cells. Conflicting results have been published as to the magnetic properties of this mineral, with Moessbauer spectroscopy indicating no magnetic ordering down to 4.2 K but density functional theory (DFT) predicting an antiferromagnetic ground state, similar to the Fe-based high-temperature superconductors with which it is isostructural and for which it is known that magnetism is suppressed by strong itinerant spin fluctuations. We investigated this latter possibility for mackinawite using photoemission spectroscopy, near-edge x-ray absorption fine structure spectroscopy, and DFT computations. Our Fe 3{sub s} core-level photoemission spectrum of mackinawite showed a clear exchange-energy splitting (2.9 eV) consistent with a 1 {micro}{sub B} magnetic moment on the Fe ions, while the Fe L-edge x-ray absorption spectrum indicated rather delocalized Fe 3{sub d} electrons in mackinawite similar to those in Fe metal. Our DFT computations demonstrated that the ground state of mackinawite is single-stripe antiferromagnetic, with an Fe magnetic moment (2.7 {micro}{sub B}) that is significantly larger than the experimental estimate and has a strong dependence on the S height and lattice parameters. All of these trends signal the existence of strong itinerant spin fluctuations. If spin fluctuations prove to be mediators of electron pairing, we conjecture that mackinawite may be one of the simplest Fe-based superconductors.
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2012-01-01
... 3 The President 1 2012-01-01 2012-01-01 false Executive Order 13573 of May 18, 2011. Blocking Property of Senior Officials of the Government of Syria 13573 Order 13573 Presidential Documents Executive Orders Executive Order 13573 of May 18, 2011 EO 13573 Blocking Property of Senior Officials of...
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2012-01-01
... 3 The President 1 2012-01-01 2012-01-01 false Executive Order 13582 of August 17, 2011. Blocking Property of the Government of Syria and Prohibiting Certain Transactions With Respect to Syria 13582 Order 13582 Presidential Documents Executive Orders Executive Order 13582 of August 17, 2011 EO 13582...
Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7
NASA Astrophysics Data System (ADS)
Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.
2012-09-01
Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.
On the zeroth-order hamiltonian for CASPT2 calculations of spin crossover compounds.
Vela, Sergi; Fumanal, Maria; Ribas-Ariño, Jordi; Robert, Vincent
2016-04-15
Complete active space self-consistent field theory (CASSCF) calculations and subsequent second-order perturbation theory treatment (CASPT2) are discussed in the evaluation of the spin-states energy difference (ΔHelec ) of a series of seven spin crossover (SCO) compounds. The reference values have been extracted from a combination of experimental measurements and DFT + U calculations, as discussed in a recent article (Vela et al., Phys Chem Chem Phys 2015, 17, 16306). It is definitely proven that the critical IPEA parameter used in CASPT2 calculations of ΔHelec , a key parameter in the design of SCO compounds, should be modified with respect to its default value of 0.25 a.u. and increased up to 0.50 a.u. The satisfactory agreement observed previously in the literature might result from an error cancellation originated in the default IPEA, which overestimates the stability of the HS state, and the erroneous atomic orbital basis set contraction of carbon atoms, which stabilizes the LS states. © 2015 Wiley Periodicals, Inc. PMID:26695936
NASA Astrophysics Data System (ADS)
Pathak, Anand; Sinha, Sitabhra
2015-09-01
Many complex systems can be represented as networks of dynamical elements whose states evolve in response to interactions with neighboring elements, noise and external stimuli. The collective behavior of such systems can exhibit remarkable ordering phenomena such as chimera order corresponding to coexistence of ordered and disordered regions. Often, the interactions in such systems can also evolve over time responding to changes in the dynamical states of the elements. Link adaptation inspired by Hebbian learning, the dominant paradigm for neuronal plasticity, has been earlier shown to result in structural balance by removing any initial frustration in a system that arises through conflicting interactions. Here we show that the rate of the adaptive dynamics for the interactions is crucial in deciding the emergence of different ordering behavior (including chimera) and frustration in networks of Ising spins. In particular, we observe that small changes in the link adaptation rate about a critical value result in the system exhibiting radically different energy landscapes, viz., smooth landscape corresponding to balanced systems seen for fast learning, and rugged landscapes corresponding to frustrated systems seen for slow learning.
Magnetization studies of the nuclear spin ordered phases of solid 3He in silver sinters
NASA Astrophysics Data System (ADS)
Schuberth, E. A.; Kath, M.; Tassini, L.; Millan-Chacartegui, C.
2005-08-01
Solid 3He, in the bcc lattice between 34 and 100 bar, exhibits two nuclear magnetic ordered phases in the sub-mK temperature range, the so called U2D2 low (magnetic) field phase and the “high field phase” above 0.4 T. To determine the exact spin structure of these phases we started a project of neutron scattering from the ordered solid in collaboration with the Hahn-Meitner Institute, Berlin, and other European and US groups. For this experiment it is crucial to grow a single crystal within the sinter needed for cooling the solid to temperatures of the order of 500 μK (or even twenty times lower in the case of the hcp lattice which is formed above 100 bar) and to keep it there long enough to measure a magnetic neutron reflection. We studied the growth of crystals in Ag sinters of different pore size and with different growth speeds to find an optimal way to obtain single crystalline samples. As a first diagnostic step we performed pulsed NMR measurements in the ordered phases of solid 3He in a sinter of 2700 Å particle size down to temperatures of 450 μK at various molar volumes. We could keep the samples in the ordered state for as long as 140 h. The second method we used was SQUID magnetometry. For the low field phase TN was indicated by a drop of the intensity, both in the NMR signal and in the dc magnetization, whereas in the high field phase an increase of about 30% was observed below the ordering temperature. For the fabrication of the sinters a packing fraction of 50% and subsequent annealing proved to be very favorable to obtain cold ordered solid. Furthermore, we find that a paramagnetic surface contribution from a few monolayers of 3He exists down to 500 μK in addition to the bulk magnetization.
NASA Astrophysics Data System (ADS)
Tessmer, Manuel; Steinhoff, Jan; Schäfer, Gerhard
2013-03-01
This paper will deal with an explicit determination of the time evolution of the spin orientation axes and the evolution of the orbital phase in the case of circular orbits under next-to-leading-order spin-orbit interactions. We modify the method of Schneider and Cui proposed [Theoreme über Bewegungsintegrale und ihre Anwendung in Bahntheorien, A Theoretische Geodäsie Vol. 121 (Verlag der Bayerischen Akademie der Wissenschaften, München, Germany, 2005)] to iteratively remove oscillatory terms in the equations of motion for different masses that were not present in the case of equal masses. Our smallness parameter is chosen to be the difference of the symmetric mass ratio to the value 1/4. Before the first Lie transformation, the set of conserved quantities consists of the total angular momentum J and the amplitudes of the orbital angular momentum and of the spins, L, S1, and S2. In contrast, S≔|S1+S2| is not conserved, and we wish to shift its nonconservation to higher orders of the smallness parameter. We perform the iterations explicitly to first order, while performing higher orders would mean no structural difference or harder mathematical difficulties. To apply this method, we develop a canonical system of spin variables reduced by the conservation law of total angular momentum, which is imposed on the phase space as a constraint. The result is an asymptotic series in ɛ that may be truncated appropriately by considering the physical properties of the regarded system.
Imprints of spin-orbit density wave in the hidden-order state of URu2Si2
NASA Astrophysics Data System (ADS)
Das, Tanmoy
2014-01-01
The mysterious second-order quantum phase transition, commonly attributed to the "hidden-order" (HO) state, in heavy-fermion metal URu2Si2 exhibits a number of paradoxical electronic and magnetic properties which cannot be associated with any conventional order parameter. We characterize and reconcile these exotic properties of the HO state based on a spin-orbit density wave order (SODW), constructed on the basis of a realistic density functional theory band structure. We quantify the nature of the gapped electronic and magnetic excitation spectrum, in agreement with measurements, while the magnetic moment is calculated to be zero owing to the spin-orbit coupling induced time-reversal invariance. Furthermore, a new collective mode in the spin-1 excitation spectrum is predicted to localize at zero momentum transfer in the HO state which can be visualized, for example, by electron spin resonance at zero magnetic field or polarized inelastic neutron scattering measurements. The results demonstrate that the concomitant broken and invariant symmetries protected SODW order not only provides insights into numerous nontrivial hidden-order phenomena, but also offers a parallel laboratory to the formation of a topologically protected quantum state beyond the quantum spin Hall state and Weyl semimetals.
Synthetic magnetic fluxes and topological order in one-dimensional spin systems
NASA Astrophysics Data System (ADS)
Graß, Tobias; Muschik, Christine; Celi, Alessio; Chhajlany, Ravindra W.; Lewenstein, Maciej
2015-06-01
Engineering topological quantum order has become a major field of physics. Many advances have been made by synthesizing gauge fields in cold atomic systems. Here we carry over these developments to other platforms which are extremely well suited for quantum engineering, namely, trapped ions and nano-trapped atoms. Since these systems are typically one-dimensional, the action of artificial magnetic fields has so far received little attention. However, exploiting the long-range nature of interactions, loops with nonvanishing magnetic fluxes become possible even in one-dimensional settings. This gives rise to intriguing phenomena, such as fractal energy spectra, flat bands with localized edge states, and topological many-body states. We elaborate on a simple scheme for generating the required artificial fluxes by periodically driving an XY spin chain. Concrete estimates demonstrating the experimental feasibility for trapped ions and atoms in wave guides are given.
Reentrant spin glass ordering in an Fe-based bulk metallic glass
Luo, Qiang; Shen, Jun
2015-02-07
We report the results of the complex susceptibility, temperature, and field dependence of DC magnetization and the nonequilibrium dynamics of a bulk metallic glass Fe{sub 40}Co{sub 8}Cr{sub 15}Mo{sub 14}C{sub 15}B{sub 6}Er{sub 2}. Solid indication of the coexistence of reentrant spin glass (SG) and ferromagnetic orderings is determined from both DC magnetization and AC susceptibility under different DC fields. Dynamics scaling of AC susceptibility indicates critical slowing down to a reentrant SG state with a static transition temperature T{sub s} = ∼17.8 K and a dynamic exponent zv = ∼7.3. The SG nature is further corroborated from chaos and memory effects, magnetic hysteresis, and aging behavior. We discuss the results in terms of the competition among random magnetic anisotropy and exchange interactions and compare them with simulation predictions.
First-order torques and solid-body spinning velocities in intense sound fields
NASA Technical Reports Server (NTRS)
Wang, T. G.; Kanber, H.; Rudnick, I.
1977-01-01
The letter reports an observation of first-order nonzero time-averaged torques and solid-body spinning velocities in intense acoustic fields. The experimental apparatus consisted of a vertical cylindrical rod supported on an air bearing and passing through a box with two loudspeakers centered on adjoining vertical sides. The rim velocity of the cylinder and the torque on the cylinder are measured as functions of air-particle velocity and the phase difference between the x and y components of the particle velocity. It is found that both rim velocity and torque are linear functions of particle velocity. Difficulties in constructing a proper theoretical description of the observed effects are discussed.
ERIC Educational Resources Information Center
Moran, K. D.
The author notes that two trends appear to be developing in litigation over the governance of the public schools. One trend is increasing participation of organized groups in suits against the schools. The other is a greater volume of litigation dealing with open meeting laws and freedom of information acts. Reflecting the second trend, the…
Code of Federal Regulations, 2013 CFR
2013-01-01
... Property of the Government of Iran and Iranian Financial Institutions 13599 Order 13599 Presidential... Government of Iran and Iranian Financial Institutions By the authority vested in me as President by the... Iran and other Iranian banks to conceal transactions of sanctioned parties, the deficiencies in...
Code of Federal Regulations, 2012 CFR
2012-01-01
.... Establishing a Coordinated Government-Wide Initiative to Promote Diversity and Inclusion in the Federal... EO 13583 Establishing a Coordinated Government-Wide Initiative to Promote Diversity and Inclusion in... opportunity, diversity, and inclusion, it is hereby ordered as follows: Section 1. Policy. Our Nation...
Order by Disorder Spin Wave Gap in the XY Pyrochlore Magnet Er2Ti2O7
NASA Astrophysics Data System (ADS)
Ross, K. A.; Qiu, Y.; Copley, J. R. D.; Dabkowska, H. A.; Gaulin, B. D.
2014-02-01
The recent determination of a robust spin Hamiltonian for the antiferromagnetic XY pyrochlore Er2Ti2O7 reveals a most convincing case of the "Order-by-Quantum-Disorder" mechanism for ground state selection. This mechanism relies on quantum fluctuations to remove an accidental symmetry of the magnetic ground state, and selects a particular ordered spin structure below TN=1.2 K. The removal of the continuous degeneracy results in an energy gap in the spectrum of spin wave excitations, long wavelength pseudo-Goldstone modes. We have measured the Order-by-Quantum-Disorder spin wave gap at a zone center in Er2Ti2O7, using low incident energy neutrons and the time-of-flight inelastic scattering method. We report a gap of Δ =0.053±0.006 meV, which is consistent with upper bounds placed on it from heat capacity measurements and roughly consistent with the theoretical estimate of ˜0.02 meV, further validating the spin Hamiltonian that led to that prediction. The gap is observed to vary with the square of the order parameter, and goes to zero for T˜TN.
NASA Astrophysics Data System (ADS)
Zhang, Q.; Singh, K.; Simon, C.; Tung, L. D.; Balakrishnan, G.; Hardy, V.
2014-07-01
The orthovanadate DyVO3 crystal, known to exhibit multiple structural, spin-, and orbital-ordering transitions, is presently investigated on the basis of magnetization, heat capacity, resistivity, dielectric, and polarization measurements. Our main result is experimental evidence for the existence of multiferroicity below a high TC of 108 K over a wide temperature range including different spin-orbital-ordered states. The onset of ferroelectricity is found to coincide with the antiferromagnetic C-type spin-ordering transition taking place at 108 K, which indicates that DyVO3 belongs to type-II multiferroics exhibiting a coupling between magnetism and ferroelectricity. Some anomalies detected on the temperature dependence of electric polarization are discussed with respect to the nature of the spin-orbital-ordered states of the V sublattice and the degree of spin alignment in the Dy sublattice. The orthovanadates RVO3 (R= rare earth or Y) form an important new category for searching for high-TC multiferroics.
Static magnetic ordering of CeCu2.1Si2 found by muon spin relaxation
NASA Technical Reports Server (NTRS)
Uemura, Y. J.; Kossler, W. J.; Yu, X. H.; Schone, H. E.; Kempton, J. R.; Stronach, C. E.; Barth, S.; Gygax, F. N.; Hitti, B.; Schenck, A.
1988-01-01
Zero- and longitudinal-field muon spin relaxation measurements on a polycrystal sample of a heavy fermion superconductor CeCu2.1 Si2 (T(c) = 0.7 K) have revealed an onset of static magnetic ordering below T approximately 0.8 K. The line shapes of the observed spectra in zero field indicate a wide distribution of static random local fields at muon sites, suggesting that the ordering is either spin glass or incommensurate spin-density-wave state. The observed width of the random local field at T = 0.05 K corresponds to a small averaged static moment of the order of 0.1 micro-B per formula unit.
Disorder from order among anisotropic next-nearest-neighbor Ising spin chains in SrHo2O4
Wen, J. -J.; Tian, W.; Garlea, V. O.; Koohpayeh, S. M.; McQueen, T. M.; Li, H. -F.; Yan, J. -Q.; Rodriguez-Rivera, J. A.; Vaknin, D.; Broholm, C. L.
2015-02-26
In this study, we describe why Ising spin chains with competing interactions in SrHo2O4 segregate into ordered and disordered ensembles at low temperatures (T). Using elastic neutron scattering, magnetization, and specific heat measurements, the two distinct spin chains are inferred to have Néel (↑↓↑↓) and double-Néel (↑↑↓↓) ground states, respectively. Below TN = 0.68(2)K, the Néel chains develop three-dimensional long range order (LRO), which arrests further thermal equilibration of the double-Néel chains so they remain in a disordered incommensurate state for T below TS = 0.52(2)K. SrHo2O4 distills an important feature of incommensurate low dimensional magnetism: kinetically trapped topological defectsmore » in a quasi–d–dimensional spin system can preclude order in d + 1 dimensions.« less
Negi, D. S. E-mail: ranjan@jncasr.ac.in; Loukya, B.; Datta, R. E-mail: ranjan@jncasr.ac.in
2015-12-07
We report on the observation of Co vacancy (V{sub Co}) induced charge ordering and ferromagnetism in CoO epitaxial thin film. The ordering is associated with the coexistence of commensurate, incommensurate, and discommensurate electronic phases. Density functional theory calculation indicates the origin of ordering in Co atoms undergoing high spin to low spin transition immediately surrounding the V{sub Co(16.6 at. %)}. Electron magnetic chiral dichroism experiment confirms the ferromagnetic signal at uncompensated Co spins. Such a native defects induced coexistence of different electronic phases at room temperature in a simple compound CoO is unique and adds to the richness of the field with the possibility of practical device application.
S. -H. Baek; Gu, G. D.; Utz, Y.; Hucker, M.; Buchner, B.; Grafe, H. -J.
2015-10-26
We report 139La nuclear magnetic resonance studies performed on a La1.875Ba0.125CuO4 single crystal. The data show that the structural phase transitions (high-temperature tetragonal → low-temperature orthorhombic → low-temperature tetragonal phase) are of the displacive type in this material. The 139La spin-lattice relaxation rate T–11 sharply upturns at the charge-ordering temperature TCO = 54 K, indicating that charge order triggers the slowing down of spin fluctuations. Detailed temperature and field dependencies of the T–11 below the spin-ordering temperature TSO=40 K reveal the development of enhanced spin fluctuations in the spin-ordered state for H ∥ [001], which are completely suppressed for largemore » fields along the CuO2 planes. Lastly, our results shed light on the unusual spin fluctuations in the charge and spin stripe ordered lanthanum cuprates.« less
NASA Astrophysics Data System (ADS)
Baek, S.-H.; Utz, Y.; Hücker, M.; Gu, G. D.; Büchner, B.; Grafe, H.-J.
2015-10-01
We report 139La nuclear magnetic resonance studies performed on a La1.875Ba0.125CuO4 single crystal. The data show that the structural phase transitions (high-temperature tetragonal→low-temperature orthorhombic→low-temperature tetragonal phase) are of the displacive type in this material. The 139La spin-lattice relaxation rate T1-1 sharply upturns at the charge-ordering temperature TCO=54 K, indicating that charge order triggers the slowing down of spin fluctuations. Detailed temperature and field dependencies of the T1-1 below the spin-ordering temperature TSO=40 K reveal the development of enhanced spin fluctuations in the spin-ordered state for H ∥[001 ] , which are completely suppressed for large fields along the CuO2 planes. Our results shed light on the unusual spin fluctuations in the charge and spin stripe ordered lanthanum cuprates.
Spin-orbit correlated magnetic order in honeycomb α-RuCl3
NASA Astrophysics Data System (ADS)
Venkataraman, Vijay Shankar; Kim, Heung-Sik; Kee, Hae-Young
2015-03-01
There has been a lot of recent interest in the combined effects of spin-orbit coupling (SOC) and electronic correlations in transition metal compounds. RuCl3 with layered honeycomb structure was proposed as a candidate material, where SOC boosts the electronic interaction, leading to an insulating phase. However, the role of SOC is not clear in materials with 4d-orbitals, since SOC strength is weaker than 5d-orbital materials. Here we study electronic band structures of honeycomb RuCl3 using ab-initio and tight binding methods, and estimate its SOC strength. We find that SOC in RuCl3 is not strong enough to justify an effective jeff = 1 / 2 single band unlike in the iridates. However, when electronic interactions are introduced, a magnetic order develops, and upper- and lower-Hubbard bands are characterized by jeff = 1 / 2 and 3 / 2 , respectively. Within a mean field theory with multi-orbital bands, we find that a zig-zag magnetic order is a ground state. Experimental implications are also discussed.
Superconductivity at the onset of spin-density-wave order in a metal.
Wang, Yuxuan; Chubukov, Andrey V
2013-03-22
We revisit the issue of superconductivity at the quantum-critical point (QCP) between a 2D paramagnet and a spin-density-wave metal with ordering momentum (π, π). This problem is highly nontrivial because the system at criticality displays a non-Fermi-liquid behavior and because the effective coupling constant λ for the pairing is generally of order one, even when the actual interaction is smaller than fermionic bandwidth. Previous study [M. A. Metlitski and S. Sachdev, Phys. Rev. B 82, 075128 (2010)] has found that the renormalizations of the pairing vertex are stronger than in BCS theory and hold in powers of log(2)(1/T). We analyze the full gap equation and argue that summing up of the leading logarithms does not lead to a pairing instability. Yet, we show that superconductivity has no threshold and appears even if λ is set to be small, because subleading logarithmical renormalizations diverge and give rise to a BCS-like result log1/T(c) ∝ 1/λ. We argue that the analogy with BCS is not accidental as at small λ superconductivity at a QCP predominantly comes from fermions that retain Fermi-liquid behavior at criticality. We compute T(c) for the actual λ ∼ O(1), and find that both Fermi-liquid and non-Fermi-liquid fermions contribute to the pairing. PMID:25166835
Spin polarized photons from an axially charged plasma at weak coupling: Complete leading order
Mamo, Kiminad A.; Yee, Ho-Ung
2016-03-24
In the presence of (approximately conserved) axial charge in the QCD plasma at finite temperature, the emitted photons are spin aligned, which is a unique P- and CP-odd signature of axial charge in the photon emission observables. We compute this “P-odd photon emission rate” in a weak coupling regime at a high temperature limit to complete leading order in the QCD coupling constant: the leading log as well as the constant under the log. As in the P-even total emission rate in the literature, the computation of the P-odd emission rate at leading order consists of three parts: (1) Comptonmore » and pair annihilation processes with hard momentum exchange, (2) soft t- and u-channel contributions with hard thermal loop resummation, (3) Landau-Pomeranchuk-Migdal resummation of collinear bremsstrahlung and pair annihilation. In conclusion, we present analytical and numerical evaluations of these contributions to our P-odd photon emission rate observable.« less
An order-by-disorder process in the cyclic phase of spin-2 condensate with a weak magnetic field
NASA Astrophysics Data System (ADS)
Zheng, Gong-Ping; Xu, Lei-Kuan; Qin, Shuai-Feng; Jian, Wen-Tian; Liang, J.-Q.
2013-07-01
We present in this paper a model study on the "order-by-disorder" process in the cyclic phase of spin-2 condensate, which forms a family of incommensurable, spiral degenerate ground states. On the basis of the ordering mechanism of entropic splitting, it is demonstrated that the energy corrections resulting from quantum fluctuations of disorder lift the accidental degeneracy of the cyclic configurations and thus lead to an eventual spiral order called the cyclic order. The order-by-disorder phenomenon is then realized even if the magnetic field exists. Finally, we show that our theoretic observations can be verified experimentally by direct detection of the cyclic order in the 87Rb condensate of a spin-2 manifold with a weak magnetic field.
Tabrizi, Shadan Ghassemi; Arbuznikov, Alexei V; Kaupp, Martin
2016-05-10
A general giant-spin Hamiltonian (GSH) describing an effective spin multiplet of an exchange-coupled metal cluster with dominant Heisenberg interactions was derived from a many-spin Hamiltonian (MSH) by treating anisotropic interactions at the third order of perturbation theory. Going beyond the existing second-order perturbation treatment allows irreducible tensor operators of rank six (or corresponding Stevens operator equivalents) in the GSH to be obtained. Such terms were found to be of crucial importance for the fitting of high-field EPR spectra of a number of single-molecule magnets (SMMs). Also, recent magnetization measurements on trigonal and tetragonal SMMs have found the inclusion of such high-rank axial and transverse terms to be necessary to account for experimental data in terms of giant-spin models. While mixing of spin multiplets by local zero-field splitting interactions was identified as the major origin of these contributions to the GSH, a direct and efficient microscopic explanation had been lacking. The third-order approach developed in this work is used to illustrate the mapping of an MSH onto a GSH for an S=6 trigonal Fe3 Cr complex that was recently investigated by high-field EPR spectroscopy. Comparisons between MSH and GSH consider the simulation of EPR data with both Hamiltonians, as well as locations of diabolical points (conical intersections) in magnetic-field space. The results question the ability of present high-field EPR techniques to determine high-rank zero-field splitting terms uniquely, and lead to a revision of the experimental GSH parameters of the Fe3 Cr SMM. Indeed, a bidirectional mapping between MSH and GSH effectively constrains the number of free parameters in the GSH. This notion may in the future facilitate spectral fitting for highly symmetric SMMs. PMID:27062248
Stoleriu, Laurentiu E-mail: cristian.enachescu@uaic.ro; Stancu, Alexandru; Enachescu, Cristian E-mail: cristian.enachescu@uaic.ro; Chakraborty, Pradip; Hauser, Andreas
2015-05-07
The recently obtained spin-crossover nanoparticles are possible candidates for applications in the recording media industry as materials for data storage, or as pressure and temperature sensors. For these applications, the intermolecular interactions and interactions between spin-crossover nanoparticles are extremely important, as they may be essential factors in triggering the transition between the two stable phases: the high-spin and low-spin ones. In order to find correlations between the distributions in size and interactions and the transition temperatures distribution, we apply the FORC (First Order Reversal Curves) method, using simulations based on a mechanoelastic model applied to 2D triangular lattices composed of molecules linked by springs and embedded in a surfactant. We consider two Gaussian distributions: one is the size of the nanoparticles and another is the elastic interactions between edge spin-crossover molecules and the surfactant molecules. In order to disentangle the kinetic and non-kinetic parts of the FORC distributions, we compare the results obtained for different temperature sweeping rates. We also show that the presence of few larger particles in a distribution centered around much smaller particles dramatically increases the hysteresis width.
An order-by-disorder process in the cyclic phase of spin-2 condensate with a weak magnetic field
Zheng, Gong-Ping; Xu, Lei-Kuan; Qin, Shuai-Feng; Jian, Wen-Tian; Liang, J.-Q.
2013-07-15
We present in this paper a model study on the “order-by-disorder” process in the cyclic phase of spin-2 condensate, which forms a family of incommensurable, spiral degenerate ground states. On the basis of the ordering mechanism of entropic splitting, it is demonstrated that the energy corrections resulting from quantum fluctuations of disorder lift the accidental degeneracy of the cyclic configurations and thus lead to an eventual spiral order called the cyclic order. The order-by-disorder phenomenon is then realized even if the magnetic field exists. Finally, we show that our theoretic observations can be verified experimentally by direct detection of the cyclic order in the {sup 87}Rb condensate of a spin-2 manifold with a weak magnetic field. -- Highlights: •A model for the order-by-disorder process in the cyclic phase of spin-2 condensate is presented. •The second-order quantum fluctuations of the mean-field states are studied. •The energy corrections lift the accidental degeneracy of the cyclic configurations. •The order-by-disorder phenomenon is realized even if a magnetic field exists. •The theoretic observations can be verified experimentally for {sup 87}Rb condensate.
Probing the coexistence of spin density wave and superconducting orders in organic superconductors
NASA Astrophysics Data System (ADS)
Narayanan, Arjun
We have conducted thermal and electrical transport measurements on the compound (TMTSF)2PF6 at temperatures down to 300 mK , magnetic fields up to 32 T and pressures up to 8 kbar. (TMTSF)2PF 6 may be tuned by pressure to exhibit a variety of low temperature ground states. From SDW at low pressures, to Superconducting metal at high pressures. In the vicinity of 6 kbar of pressure, samples show on cooling, first a SDW phase transition and then superconductivity. This coexistence of two transitions, is also seen in other material classes, for example, The Pnictides and the Heavy fermion superconductors. While in those classes the physics of simultaneous competing orders is not easy to explore, in (TMTSF)2PF 6 , owing in part to its remarkably reliable crystal growth, and its simple yet feature rich electronic structure, the situation is now clearer. Simultaneous resistivity and thermopower measurements under pressure along all three crystal axes, provide evidence for phase separation between SDW and metallic domains. The pressure evolution of the phase boundaries may also be qualitatively followed. The metallic domains in coexistence are identi ed as the high pressure metal phase by a variety of signatures in magnetoresistance( the presence of Field induced Spin density waves, Rapid oscillations, the Lebed oscillations and Danner-Chaikin-Kang oscillations.) The main result of this thesis is a characterisation of the coexistence state that allows us to eliminate various theoretical models and assert that the result of interacting SDW and Metallic orders is a phase separation into large scale domains with domain widths of the order of micrometers in these salts. Further that the domain walls follow a well defined geometry linked to the geometry of the lattice.
Development of multi-mode diabatic spin-orbit models at arbitrary order
NASA Astrophysics Data System (ADS)
Weike, Thomas; Eisfeld, Wolfgang
2016-03-01
The derivation of diabatic spin-orbit (SO) Hamiltonians is presented, which are expanded in terms of nuclear coordinates to arbitrary order including the treatment of multi-mode systems, having more than one mode of the same symmetry. The derivation is based on the microscopic Breit-Pauli SO operator and the consequent utilization of time reversal and spatial symmetry transformation properties of basis functions and coordinates. The method is demonstrated for a set of 2E and 2A1 states in C3 v ∗ (double group) symmetry, once for a 3D case of one a1 and one e mode and once for a 9D case of three a1 and three e coordinates. It is shown that the general structure of the diabatic SO Hamiltonian only depends on the basis states and is strictly imposed by time reversal symmetry. The resulting matrix can be expressed easily by a power series using six parametrized structure matrices as expansion coefficients multiplied by the associated monomials in terms of symmetrized coordinates. The explicit example presented here provides a full-dimensional diabatic SO model for methyl halide cations, which will be studied in the future.
NASA Astrophysics Data System (ADS)
Casanova, David; Rhee, Young Min; Head-Gordon, Martin
2008-04-01
Scaled opposite spin (SOS) second order perturbative corrections to single excitation configuration interaction (CIS) are extended to correctly treat quasidegeneracies between excited states. Two viable methods, termed as SOS-CIS(D0) and SOS-CIS(D1), are defined, implemented, and tested. Each involves one empirical parameter (plus a second for the SOS-MP2 ground state), has computational cost that scales with the fourth power of molecule size, and has storage requirements that are cubic, with only quantities of the rank of single excitations produced and stored during iterations. Tests on a set of low-lying adiabatic valence excitation energies and vertical Rydberg excitations of organic and inorganic molecules show that the empirical parameter can be acceptably transferred from the corresponding nondegenerate perturbation theories without any further fitting. Further tests on higher excited states show that the new methods correctly perform for surface crossings for which nondegenerate approaches fail. Numerical results show that SOS-CIS(D0) appears to treat Rydberg excitations in a more balanced way than SOS-CIS(D1) and is, therefore, likely to be the preferred approach. It should be useful for exploring excited state geometries, transition structures, and conical intersections for states of medium to large organic molecules that are dominated by single excitations.
Code of Federal Regulations, 2014 CFR
2014-01-01
... 10 Energy 4 2014-01-01 2014-01-01 false Applicable Federal Statutes, Executive Orders, and Government-wide Regulations A Appendix A to Part 603 Energy DEPARTMENT OF ENERGY (CONTINUED) ASSISTANCE REGULATIONS TECHNOLOGY INVESTMENT AGREEMENTS Pt. 603, App. A Appendix A to Part 603—Applicable Federal Statutes, Executive Orders, and...
The stability of steady motion of magnetic domain wall: Role of higher-order spin-orbit torques
He, Peng-Bin Yan, Han; Cai, Meng-Qiu; Li, Zai-Dong
2015-12-14
The steady motion of magnetic domain wall driven by spin-orbit torques is investigated analytically in the heavy/ferromagnetic metal nanowires for three cases with a current transverse to the in-plane and perpendicular easy axis, and along the in-plane easy axis. By the stability analysis of Walker wall profile, we find that if including the higher-order spin-orbit torques, the Walker breakdown can be avoided in some parameter regions of spin-orbit torques with a current transverse to or along the in-plane easy axis. However, in the case of perpendicular anisotropy, even considering the higher-order spin-orbit torques, the velocity of domain wall cannot be efficiently enhanced by the current. Furthermore, the direction of wall motion is dependent on the configuration and chirality of domain wall with a current along the in-plane easy axis or transverse to the perpendicular one. Especially, the direction of motion can be controlled by the initial chirality of domain wall. So, if only involving the spin-orbit mechanism, it is preferable to adopt the scheme of a current along the in-plane easy axis for enhancing the velocity and controlling the direction of domain wall.
The stability of steady motion of magnetic domain wall: Role of higher-order spin-orbit torques
NASA Astrophysics Data System (ADS)
He, Peng-Bin; Yan, Han; Cai, Meng-Qiu; Li, Zai-Dong
2015-12-01
The steady motion of magnetic domain wall driven by spin-orbit torques is investigated analytically in the heavy/ferromagnetic metal nanowires for three cases with a current transverse to the in-plane and perpendicular easy axis, and along the in-plane easy axis. By the stability analysis of Walker wall profile, we find that if including the higher-order spin-orbit torques, the Walker breakdown can be avoided in some parameter regions of spin-orbit torques with a current transverse to or along the in-plane easy axis. However, in the case of perpendicular anisotropy, even considering the higher-order spin-orbit torques, the velocity of domain wall cannot be efficiently enhanced by the current. Furthermore, the direction of wall motion is dependent on the configuration and chirality of domain wall with a current along the in-plane easy axis or transverse to the perpendicular one. Especially, the direction of motion can be controlled by the initial chirality of domain wall. So, if only involving the spin-orbit mechanism, it is preferable to adopt the scheme of a current along the in-plane easy axis for enhancing the velocity and controlling the direction of domain wall.
On the definition of the spin-free cumulant of the second-order reduced density matrix
NASA Astrophysics Data System (ADS)
Lain, Luis; Torre, Alicia; Bochicchio, Roberto
2002-09-01
This note deals with the appropriate definition for the spin-free cumulant of the second-order reduced density matrix. Our approach leads to a direct derivation of one of the proposals reported by Kutzelnigg and Mukherjee [J. Chem. Phys. 116, 4787 (2002)] and it points out its suitability.
Magnetic ordering in the ultrapure site-diluted spin chain materials SrCu1 -xNixO2
NASA Astrophysics Data System (ADS)
Simutis, G.; Thede, M.; Saint-Martin, R.; Mohan, A.; Baines, C.; Guguchia, Z.; Khasanov, R.; Hess, C.; Revcolevschi, A.; Büchner, B.; Zheludev, A.
2016-06-01
The muon spin rotation technique is used to study magnetic ordering in ultrapure samples of SrCu1 -xNixO2 , an archetypical S =1 /2 antiferromagnetic Heisenberg chain system with a small number of S =1 defects. The ordered state in the parent compound is shown to be highly homogeneous, contrary to a previous report [M. Matsuda et al., Phys. Rev. B 55, R11953 (1997), 10.1103/PhysRevB.55.R11953]. Even a minute number of Ni impurities results in inhomogeneous order and a decrease of the transition temperature. At as little as 0.5 % Ni concentration, magnetic ordering is entirely suppressed. The results are compared to previous theoretical studies of weakly coupled spin chains with site defects.
NASA Astrophysics Data System (ADS)
Vladimirov, A. A.; Ihle, D.; Plakida, N. M.
2015-02-01
The spin-wave excitation spectrum, magnetization, and Néel temperature for the quasi-two-dimensional spin-1/2 antiferromagnetic Heisenberg model with the compass-model interaction in the plane proposed for iridates are calculated in the random phase approximation. The spin-wave spectrum agrees well with data of Lanczos diagonalization. We find that the Néel temperature is enhanced by the compass-model interaction and is close to the experimental value for Ba2IrO4.
Bigdeli, M.; Bordbar, G. H.; Poostforush, A.
2010-09-15
The lowest order constrained variational technique has been used to investigate some of the thermodynamic properties of spin-polarized hot asymmetric nuclear matter, such as the free energy, symmetry energy, susceptibility, and equation of state. We have shown that the symmetry energy of the nuclear matter is substantially sensitive to the value of spin polarization. Our calculations show that the equation of state of the polarized hot asymmetric nuclear matter is stiffer for higher values of the polarization as well as the isospin asymmetry parameter. Our results for the free energy and susceptibility show that spontaneous ferromagnetic phase transition cannot occur for hot asymmetric matter.
Magnetic damping and spin polarization of highly ordered B2 Co2FeAl thin films
NASA Astrophysics Data System (ADS)
Cui, Yishen; Lu, Jiwei; Schäfer, Sebastian; Khodadadi, Behrouz; Mewes, Tim; Osofsky, Mike; Wolf, Stuart A.
2014-08-01
Epitaxial Co2FeAl films were synthesized using the Biased Target Ion Beam Deposition technique. Post annealing yielded Co2FeAl films with an improved B2 chemical ordering. Both the magnetization and the Gilbert damping parameter were reduced with increased B2 ordering. A low damping parameter, ˜0.002, was attained in B2 ordered Co2FeAl films without the presence of the L21 Heusler phase, which suggests that the B2 structure is sufficient for providing low damping in Co2FeAl. The spin polarization was ˜53% and was insensitive to the chemical ordering.
Effective spin-1/2 scalar chiral order on kagome lattices in Nd3Sb3Mg2O14
NASA Astrophysics Data System (ADS)
Scheie, A.; Sanders, M.; Krizan, J.; Qiu, Y.; Cava, R. J.; Broholm, C.
2016-05-01
We introduce Nd3Sb3Mg2O14 with ideal kagome lattices of neodymium ions in ABC stacking. Thermodynamic measurements show a Curie-Weiss temperature of ΘCW=-0.12 K, a Nd3 + spin-1/2 Kramers doublet ground state, and a second-order phase transition at TN=0.56 (2 ) K. Neutron scattering reveals noncoplanar scalar chiral k =0 magnetic order with a correlation length exceeding 400 Å=55 a and an ordered moment of 1.79 (5 ) μB . This order includes a canted ferromagnetic component perpendicular to the kagome planes favored by Dzyaloshinskii-Moriya interactions.
Antiferromagnetic order in a semiconductor quantum well with spin-orbit coupling
NASA Astrophysics Data System (ADS)
Marinescu, D. C.
2015-05-01
An argument is made on the existence of a low-temperature itinerant antiferromagnetic (AF) spin alignment, rather than persistent helical (PH), in the ground state of a two dimensional electron gas in a semiconductor quantum well with linear spin-orbit Rashba-Dresselhaus interaction at equal coupling strengths, α. This result is obtained on account of the opposite-spin single-particle state degeneracy at k = 0 that makes the spin instability possible. A theory of the resulting magnetic phase is formulated within the Hartree-Fock approximation of the Coulomb interaction. In the AF state the direction of the fractional polarization is obtained to be aligned along the displacement vector of the single-particle states.
Plötzing, M; Adam, R; Weier, C; Plucinski, L; Eich, S; Emmerich, S; Rollinger, M; Aeschlimann, M; Mathias, S; Schneider, C M
2016-04-01
The fundamental mechanism responsible for optically induced magnetization dynamics in ferromagnetic thin films has been under intense debate since almost two decades. Currently, numerous competing theoretical models are in strong need for a decisive experimental confirmation such as monitoring the triggered changes in the spin-dependent band structure on ultrashort time scales. Our approach explores the possibility of observing femtosecond band structure dynamics by giving access to extended parts of the Brillouin zone in a simultaneously time-, energy- and spin-resolved photoemission experiment. For this purpose, our setup uses a state-of-the-art, highly efficient spin detector and ultrashort, extreme ultraviolet light pulses created by laser-based high-order harmonic generation. In this paper, we present the setup and first spin-resolved spectra obtained with our experiment within an acquisition time short enough to allow pump-probe studies. Further, we characterize the influence of the excitation with femtosecond extreme ultraviolet pulses by comparing the results with data acquired using a continuous wave light source with similar photon energy. In addition, changes in the spectra induced by vacuum space-charge effects due to both the extreme ultraviolet probe- and near-infrared pump-pulses are studied by analyzing the resulting spectral distortions. The combination of energy resolution and electron count rate achieved in our setup confirms its suitability for spin-resolved studies of the band structure on ultrashort time scales. PMID:27131684
NASA Astrophysics Data System (ADS)
Plötzing, M.; Adam, R.; Weier, C.; Plucinski, L.; Eich, S.; Emmerich, S.; Rollinger, M.; Aeschlimann, M.; Mathias, S.; Schneider, C. M.
2016-04-01
The fundamental mechanism responsible for optically induced magnetization dynamics in ferromagnetic thin films has been under intense debate since almost two decades. Currently, numerous competing theoretical models are in strong need for a decisive experimental confirmation such as monitoring the triggered changes in the spin-dependent band structure on ultrashort time scales. Our approach explores the possibility of observing femtosecond band structure dynamics by giving access to extended parts of the Brillouin zone in a simultaneously time-, energy- and spin-resolved photoemission experiment. For this purpose, our setup uses a state-of-the-art, highly efficient spin detector and ultrashort, extreme ultraviolet light pulses created by laser-based high-order harmonic generation. In this paper, we present the setup and first spin-resolved spectra obtained with our experiment within an acquisition time short enough to allow pump-probe studies. Further, we characterize the influence of the excitation with femtosecond extreme ultraviolet pulses by comparing the results with data acquired using a continuous wave light source with similar photon energy. In addition, changes in the spectra induced by vacuum space-charge effects due to both the extreme ultraviolet probe- and near-infrared pump-pulses are studied by analyzing the resulting spectral distortions. The combination of energy resolution and electron count rate achieved in our setup confirms its suitability for spin-resolved studies of the band structure on ultrashort time scales.
NASA Astrophysics Data System (ADS)
Harrison, Richard J.
2009-02-01
Magnetic ordering in the ilmenite-hematite solid solution (Fe2-xTixO3) has been investigated using Monte Carlo simulations, with particular emphasis on the low-temperature spin glass region of the phase diagram. Complex magnetic behavior is observed due to the presence of two competing magnetic order parameters: a "hematite-like" ordering with a two-layer repeat (Q2) and an "ilmenite-like" ordering with a four-layer repeat (Q4). The susceptibility and degree of magnetic order were calculated from the Fourier transform of the layer-averaged spin distribution, allowing long-range and short-range contributions from Q2 and Q4 to be analyzed separately. For x < 0.8, the ferrimagnetic (FM) phase remains stable down to 0 K. For x ≥ 0.8 a heterogeneous FM phase (HFM) followed by a modulated FM phase (MFM) develops. There is an increasing contribution from Q4 with increasing x, and a pronounced cusp in both Q2 and Q4 susceptibilities develops at 30 K. The superposition of Q2 and Q4 leads to frustrated layers containing dynamically disordered spins. Freezing of this spin disorder below 30 K is responsible for the cusp in susceptibility, which can be classified as a reentrant spin glass (RSG) transition. A gradual loss of long-range FM order occurs as the percolation threshold is approached, resulting in a conventional spin glass (CSG) with no long-range order below 30 K for x ≥ 0.92. For x > 0.95, a transition to an antiferromagnetic (AF) phase occurs at 40-55 K, followed by an RSG transition at 20-30 K. Changes to the phase diagram caused by chemical clustering are determined using a preannealing algorithm. Clustering expands the AF field to x > 0.9 and the HFM field to x ≥ 0.55. The topology of the simulated phase diagram compares favorably with experiments but suggests that the nature of some phase boundaries should be reexamined from both experimental and computational perspectives.
48 CFR 252.251-7000 - Ordering from Government supply sources.
Code of Federal Regulations, 2010 CFR
2010-10-01
..., for automated data processing equipment, software and maintenance, communications equipment and... below: Contractor's Billing Address (include point of contact and telephone number): Government Remittance Address (include point of contact and telephone number): (End of clause)...
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2014-10-01
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ERIC Educational Resources Information Center
Parente, Roberto; Feola, Rosangela; Petrone, Michele
2011-01-01
This paper reports an investigation of governance issues in Italian academic spin-offs that arise from the need to balance the powers of two categories of partner: academic inventors and external investors (such as established companies and venture capital funds). The relationship between inventors and external investors, jointly pursuing a…
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... Order AGENCY: Consumer Product Safety Commission. ACTION: Notice. ] SUMMARY: It is the policy of the Commission to publish settlements which it provisionally accepts under the Consumer Product Safety Act in the... that TMG is harmful if swallowed, and that, upon ingestion, it targets the kidneys and central...
Damped spin waves in the intermediate ordered phases in Ni_{3}V_{2}O_{8}
Ehlers, Georg; Podlesnyak, Andrey A.; Frontzek, Matthias D.; Pushkarev, A. V.; Shiryaev, Sergie V.; Barilo, Sergie
2015-06-09
Here, spin dynamics in the intermediate ordered phases (between 4 and 9 K) in Ni_{3}V_{2}O_{8} have been studied with inelastic neutron scattering. It is found that the spin waves are very diffuse, indicative of short lived correlations and the coexistence of paramagnetic moments with the long-range ordered state.
Long-range orders and spin/orbital freezing in the two-band Hubbard model
NASA Astrophysics Data System (ADS)
Steiner, Karim; Hoshino, Shintaro; Nomura, Yusuke; Werner, Philipp
2016-08-01
We solve the orbitally degenerate two-band Hubbard model within dynamical mean field theory and map out the instabilities to various symmetry-broken phases based on an analysis of the corresponding lattice susceptibilities. Phase diagrams as a function of the Hund coupling parameter J are obtained both for the model with rotationally invariant interaction and for the model with Ising-type anisotropy. For negative J , an intraorbital spin-singlet superconducting phase appears at low temperatures, while the normal state properties are characterized by an orbital-freezing phenomenon. This is the negative-J analog of the recently discovered fluctuating-moment induced s -wave spin-triplet superconductivity in the spin-freezing regime of multiorbital models with J >0 .
Dispersionless Spin Waves and Underlying Field-Induced Magnetic Order in Gadolinium Gallium Garnet.
d'Ambrumenil, N; Petrenko, O A; Mutka, H; Deen, P P
2015-06-01
We report the results of neutron diffraction and inelastic neutron scattering on a powder sample of Gd_{3}Ga_{5}O_{12} at high magnetic fields. Analysis of the diffraction data shows that in high fields (B≳1.8 T) the spins are not fully aligned, but are canted slightly as a result of the dipolar interaction. The magnetic phase for fields ≲1.8 T is characterized by antiferromagnetic peaks at (210) and an incommensurate wave vector. The dominant contribution to inelastic scattering at large momentum transfers is from a band of almost dispersionless excitations. We show that these correspond to the spin waves localized on ten site rings, expected on the basis of nearest neighbor exchange interaction, and that the spectrum at high fields B≳1.8 T is well described by a spin wave theory. PMID:26196642
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2011-01-01
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Orbital-spin order and the origin of structural distortion in MgTi2O4
NASA Astrophysics Data System (ADS)
Leoni, S.; Yaresko, A. N.; Perkins, N.; Rosner, H.; Craco, L.
2008-09-01
We analyze electronic, magnetic, and structural properties of the spinel compound MgTi2O4 using the local-density approximation+U method. We show how MgTi2O4 undergoes to a canted orbital-spin ordered state, where charge, spin, and orbital degrees of freedom are frozen in a geometrically frustrated network by electron interactions. In our picture orbital order stabilizes the magnetic ground state and controls the degree of structural distortions. The latter is dynamically derived from the cubic structure in the correlated LDA+U potential. Our ground-state theory provides a consistent picture for the dimerized phase of MgTi2O4 , and might be applicable to frustrated materials in general.
NASA Astrophysics Data System (ADS)
Wang, Qing-Wei; Liu, Da-Yong; Quan, Ya-Min; Zou, Liang-Jian
2016-08-01
We theoretically study the coexistence of spin density wave (SDW) and superconductivity (SC) in ironpnictide superconductors based on a three-orbital model, focusing on the momentum-space and real-space distributions of SDW and SC order parameters in the coexistence region. We show that a SDW-SC coexisting state lies in the T-n phase diagram, in qualitative agreement with those of NaFe1 - xCoxAs and Ba(Fe1 - xCox)2As2. In the SC state the pairing wavefunction has s± symmetry with sx2y2 and sx2+y2 components. In the coexisting state, the SDW and SC order parameters display strong orbital-selective competitions in momentum space, which also result in real-space modulation and spin singlet-triplet mixing in the Cooper pairing amplitude. We expect that the obtained features may be observed in future experiments.
Size-dependent magnetic ordering and spin-dynamics in DyPO4 and GdPO4 nanoparticles
Evangelisti, Marco; Sorop, Tibi G; Bakharev, Oleg N; Visser, Dirk; Hillier, Adrian D.; Alonso, Juan; Haase, Markus; Boatner, Lynn A; De Jongh, L. Jos
2011-01-01
Low-temperature magnetic susceptibility and heat capacity measurements on nanoparticles (d 2.6 nm) of the antiferromagnetic compounds DyPO4 (TN = 3:4 K) and GdPO4 (TN = 0:77 K) provide clear demonstrations of finite-size effects, which limit the divergence of the magnetic correlation lengths, thereby suppressing the bulk long-range magnetic ordering transitions. Instead, the incomplete antiferromagnetic order inside the particles leads to the formation of net magnetic moments on the particles. For the nanoparticles of Ising-type DyPO4 superparamagnetic blocking is found in the ac-susceptibility at 1 K, those of the XY-type GdPO4 analogue show a dipolar spin-glass transition at 0:2 K. Monte Carlo simulations for the magnetic heat capacities of both bulk and nanoparticle samples are in agreement with the experimental data. Strong size effects are also apparent in the Dy3+ and Gd3+ spin-dynamics, which were studied by zero-field SR relaxation and high-field 31P-NMR nuclear relaxation measurements. The freezing transitions observed in the ac-susceptibility of the nanoparticles also appear as peaks in the temperature dependence of the zero-field SR rates, but at slightly higher temperatures - as to be expected from the higher frequency of the muon probe. For both bulk and nanoparticles of GdPO4, the muon and 31P-NMR rates are for T 5 K dominated by exchange-narrowed hyperfine broadening arising from the electron spin-spin interactions inside the particles. The dipolar hyperfine interactions acting on the muons and the 31P are, however, much reduced in the nanoparticles. For the DyPO4 analogues the high-temperature rates appear to be fully determined by electron spin-lattice relaxation processes.
NASA Astrophysics Data System (ADS)
Wu, Ya-Jie; Li, Ning; He, Jing; Kou, Su-Peng
2016-03-01
In this paper, based on mean-field approach and random-phase-approximation, we study the magnetic properties of the repulsive Haldane-Hubbard model on a square lattice. We find antiferromagnetic order driven topological spin density waves beyond Landau’s symmetry-breaking paradigm, for which the effective low energy physics is determined by Chern-Simons-Hopf gauge field theories with different K matrices.
Libery, Order and Justice: An Introduction to the Constitutional Principles of American Government.
ERIC Educational Resources Information Center
McClellan, James
This publication on the constitutional principles of the U.S. Government consists of the textbook and teacher's guide. The textbook begins with a review of constitutionalism in antiquity, in early modern England, and in colonial America. Following sections outline the constitutional convention in Philadelphia, the principles of the constitution,…
NASA Astrophysics Data System (ADS)
Lewoczko, April D.
In part I, we investigate gold catalysis in the chemistry of organonitrogen compounds. We examine the adsorption of oxygen, nitrogen and sulfur atoms on the gold (111), (100) and (211) surfaces using density functional theory (DFT). Sulfur atoms bind most strongly, followed by oxygen and nitrogen atoms with stronger adsorption for greater coordination to the surface. We see a trend of stronger adsorption to undercoordinated gold, but find it is non-universal with the adsorption strength trend: (111) > (211) > (100). We consider the diffusion of oxygen, nitrogen and sulfur adatoms and find facile long-range diffusion of oxygen atoms on the (100) surface. Lastly, we compare the adsorption of methylamine on gold to that of a selection of alkylamines, methanol and methanethiol. In each case, the ontop site is preferred with stronger adsorption at low coordinated gold. At oxygen atom coverages of 0.125 -- 0.25 ML on Au (111), we find cooperative adsorption of methylamine and oxygen atoms. Energetic costs for adsorbate tilt from the surface normal and rotation about the gold-nitrogen bond are calculated. While methylamine rotation is barrierless on the (111) and (211) surfaces, it has a low energetic barrier for the 0.125 ML and 0.25 ML O atom pre-covered Au (111) surfaces. In part II, we interpret the experimental mass spectrum of small gas phase manganese sulfide clusters using DFT and elucidate the role of ionicity and spin ordering in sizes with special stability, i.e. magic clusters. We first consider nine low lying minima (MnS)6 structures and reveal antiferromagnetic (AFM) spin ordering with a ˜0.1 eV/pair AFM energy benefit and a ˜0.1 A shrinkage of average Mn-Mn distances over clusters with ferromagnetic (FM) spin ordering. We calculate energetic barriers for interconversion between the two lowest lying (MnS)6 isomers and predict an elevated cluster melting temperature due to increased configurational entropy in a pre-melted state. Second, we demonstrate the
Spin dynamics, short range order and spin freezing in Y0.5Ca0.5BaCo4O7
Stewart, John Ross; Ehlers, Georg; Fouquet, Peter; Mutka, Hannu; Payen, Christophe; Lortz, Rolf
2011-01-01
Y0.5Ca0.5BaCo4O7 was recently introduced as a possible candidate for capturing some of the predicted classical spin kagome ground-state features. Stimulated by this conjecture, we have taken up a more complete study of the spin correlations in this compound with neutron scattering methods on a powder sample characterized with high-resolution neutron diffraction and the temperature dependence of magnetic susceptibility and specific heat. We have found that the frustrated near-neighbor magnetic correlations involve not only the kagome planes but concern the full Co sublattice, as evidenced by the analysis of the wave-vector dependence of the short-range order. We conclude from our results that the magnetic moments are located on the Co sublattice as a whole and that correlations extend beyond the two-dimensional kagome planes. We identify intriguing dynamical properties, observing high-frequency fluctuations with a Lorentzian linewidth G?20 meV at ambient temperature. On cooling a low-frequency ({approx}1 meV) dynamical component develops alongside the high-frequency fluctuations, which eventually becomes static at temperatures below T {approx} 50 K. The high-frequency response with an overall linewidth of {approx}10 meV prevails at T?2 K, coincident with a fully elastic short-range-ordered contribution.
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Spin-driven ordering of Cr in the equiatomic high entropy alloy NiFeCrCo
NASA Astrophysics Data System (ADS)
Niu, C.; Zaddach, A. J.; Oni, A. A.; Sang, X.; Hurt, J. W.; LeBeau, J. M.; Koch, C. C.; Irving, D. L.
2015-04-01
Spin-driven ordering of Cr in an equiatomic fcc NiFeCrCo high entropy alloy (HEA) was predicted by first-principles calculations. Ordering of Cr is driven by the reduction in energy realized by surrounding anti-ferromagnetic Cr with ferromagnetic Ni, Fe, and Co in an alloyed L12 structure. The fully Cr-ordered alloyed L12 phase was predicted to have a magnetic moment that is 36% of that for the magnetically frustrated random solid solution. Three samples were synthesized by milling or casting/annealing. The cast/annealed sample was found to have a low temperature magnetic moment that is 44% of the moment in the milled sample, which is consistent with theoretical predictions for ordering. Scanning transmission electron microscopy measurements were performed and the presence of ordered nano-domains in cast/annealed samples throughout the equiatomic NiFeCrCo HEA was identified.
Spin-driven ordering of Cr in the equiatomic high entropy alloy NiFeCrCo
Niu, C.; Zaddach, A. J.; Oni, A. A.; Sang, X.; LeBeau, J. M.; Koch, C. C.; Irving, D. L.; Hurt, J. W.
2015-04-20
Spin-driven ordering of Cr in an equiatomic fcc NiFeCrCo high entropy alloy (HEA) was predicted by first-principles calculations. Ordering of Cr is driven by the reduction in energy realized by surrounding anti-ferromagnetic Cr with ferromagnetic Ni, Fe, and Co in an alloyed L1{sub 2} structure. The fully Cr-ordered alloyed L1{sub 2} phase was predicted to have a magnetic moment that is 36% of that for the magnetically frustrated random solid solution. Three samples were synthesized by milling or casting/annealing. The cast/annealed sample was found to have a low temperature magnetic moment that is 44% of the moment in the milled sample, which is consistent with theoretical predictions for ordering. Scanning transmission electron microscopy measurements were performed and the presence of ordered nano-domains in cast/annealed samples throughout the equiatomic NiFeCrCo HEA was identified.
NASA Astrophysics Data System (ADS)
Calderón Bustillo, Juan; Husa, Sascha; Sintes, Alicia M.; Pürrer, Michael
2016-04-01
Current template-based gravitational wave searches for compact binary coalescences use waveform models that omit the higher order modes content of the gravitational radiation emitted, considering only the quadrupolar (ℓ,|m |)=(2 ,2 ) modes. We study the effect of such omission for the case of aligned-spin compact binary coalescence searches for equal-spin (and nonspinning) binary black holes in the context of two versions of Advanced LIGO: the upcoming 2015 version, known as early Advanced LIGO (eaLIGO) and its zero-detuned high-energy power version, which we will refer to as Advanced LIGO (AdvLIGO). In addition, we study the case of a nonspinning search for initial LIGO (iLIGO). We do this via computing the effectualness of the aligned-spin SEOBNRv1 reduced order model waveform family, which only considers quadrupolar modes, toward hybrid post-Newtonian/numerical relativity waveforms which contain higher order modes. We find that for all LIGO versions losses of more than 10% of events occur in the case of AdvLIGO for mass ratio q ≥6 and total mass M ≥100 M⊙ due to the omission of higher modes, this region of the parameter space being larger for eaLIGO and iLIGO. Moreover, while the maximum event loss observed over the explored parameter space for AdvLIGO is of 15% of events, for iLIGO and eaLIGO, this increases up to (39,23)%. We find that omission of higher modes leads to observation-averaged systematic parameter biases toward lower spin, total mass, and chirp mass. For completeness, we perform a preliminar, nonexhaustive comparison of systematic biases to statistical errors. We find that, for a given signal-to-noise ratio, systematic biases dominate over statistical errors at much lower total mass for eaLIGO than for AdvLIGO.
Vekic, M.; Cannon, J.W.; Scalapino, D.J.; Scalettar, R.T.; Sugar, R.L. Physics Department, Centenary College, 2911 Centenary Boulevard, Shreveport, Louisiana 71104 Department of Physics, University of California, Santa Barbara, California 93106 )
1995-03-20
We study the two-dimensional periodic Anderson model at half filling using quantum Monte Carlo (QMC) techniques. The ground state undergoes a magnetic order-disorder transition as a function of the effective exchange coupling between the conduction and localized bands. Low-lying spin and charge excitations are determined using the maximum entropy method to analytically continue the QMC data. At finite temperature we find a competition between the Kondo effect and antiferromagnetic order which develops in the localized band through Ruderman-Kittel-Kasuya-Yosida interactions.
NASA Astrophysics Data System (ADS)
Kardash, Maria E.; Dzuba, Sergei A.
2014-12-01
Lipid-cholesterol interactions are responsible for different properties of biological membranes including those determining formation in the membrane of spatial inhomogeneities (lipid rafts). To get new information on these interactions, electron spin echo (ESE) spectroscopy, which is a pulsed version of electron paramagnetic resonance (EPR), was applied to study 3β-doxyl-5α-cholestane (DCh), a spin-labeled analog of cholesterol, in phospholipid bilayer consisted of equimolecular mixture of 1,2-dipalmitoyl-sn-glycero-3-phosphocholine and 1,2-dioleoyl-sn-glycero-3-phosphocholine. DCh concentration in the bilayer was between 0.1 mol.% and 4 mol.%. For comparison, a reference system containing a spin-labeled 5-doxyl-stearic acid (5-DSA) instead of DCh was studied as well. The effects of "instantaneous diffusion" in ESE decay and in echo-detected (ED) EPR spectra were explored for both systems. The reference system showed good agreement with the theoretical prediction for the model of spin labels of randomly distributed orientations, but the DCh system demonstrated remarkably smaller effects. The results were explained by assuming that neighboring DCh molecules are oriented in a correlative way. However, this correlation does not imply the formation of clusters of cholesterol molecules, because conventional continuous wave EPR spectra did not show the typical broadening due to aggregation of spin labels and the observed ESE decay was not faster than in the reference system. So the obtained data evidence that cholesterol molecules at low concentrations in biological membranes can interact via large distances of several nanometers which results in their orientational self-ordering.
Kardash, Maria E.; Dzuba, Sergei A.
2014-12-07
Lipid-cholesterol interactions are responsible for different properties of biological membranes including those determining formation in the membrane of spatial inhomogeneities (lipid rafts). To get new information on these interactions, electron spin echo (ESE) spectroscopy, which is a pulsed version of electron paramagnetic resonance (EPR), was applied to study 3β-doxyl-5α-cholestane (DCh), a spin-labeled analog of cholesterol, in phospholipid bilayer consisted of equimolecular mixture of 1,2-dipalmitoyl-sn-glycero-3-phosphocholine and 1,2-dioleoyl-sn-glycero-3-phosphocholine. DCh concentration in the bilayer was between 0.1 mol.% and 4 mol.%. For comparison, a reference system containing a spin-labeled 5-doxyl-stearic acid (5-DSA) instead of DCh was studied as well. The effects of “instantaneous diffusion” in ESE decay and in echo-detected (ED) EPR spectra were explored for both systems. The reference system showed good agreement with the theoretical prediction for the model of spin labels of randomly distributed orientations, but the DCh system demonstrated remarkably smaller effects. The results were explained by assuming that neighboring DCh molecules are oriented in a correlative way. However, this correlation does not imply the formation of clusters of cholesterol molecules, because conventional continuous wave EPR spectra did not show the typical broadening due to aggregation of spin labels and the observed ESE decay was not faster than in the reference system. So the obtained data evidence that cholesterol molecules at low concentrations in biological membranes can interact via large distances of several nanometers which results in their orientational self-ordering.
DOUBLE TRANSVERSE SPIN ASYMMETRIES AT NEXT-TO-LEADING ORDER IN QCD.
MUKHERJEE,A.; STRATMANN,M.; VOGELSANG,W.
2004-10-10
We present a technique to calculate the cross sections and spin asymmetries for transversely polarized pp collisions at NLO in QCD and report on the use of this technique for the processes p{up_arrow}p{up_arrow} {yields} {gamma}X, p{up_arrow}p{up_arrow} {yields} {pi}X and p{up_arrow}p{up_arrow} {yields} {ell}{sup +}{ell}{sup -} X.
Spin and orbital ordering in Y_{1-x}La_{x}VO₃
Yan, J.-Q.; Zhou, J.-S.; Cheng, J. G.; Goodenough, J. B.; Ren, Y.; Llobet, A.; McQueeney, R. J.
2011-12-02
The spin and orbital ordering in Y_{1-x}La_{x}VO₃ (0.30 ≤ x ≤ 1.0) has been studied to map out the phase diagram over the whole doping range 0 ≤ x ≤ 1. The phase diagram is compared with that for RVO₃ (R = rare earth or Y) perovskites without A-site variance. For x > 0.20, no long-range orbital ordering was observed above the magnetic ordering temperature T_{N}; the magnetic order is accompanied by a lattice anomaly at a Tt ≤ T_{N} as in LaVO₃. The magnetic ordering below Tt ≤ T_{N} is G type in the compositional range 0.20 ≤ x ≤ 0.40 and C type in the range 0.738 ≤ x ≤ 1.0. Magnetization and neutron powder diffraction measurements point to the coexistence below T_{N} of the two magnetic phases in the compositional range 0.4 < x < 0.738. Samples in the compositional range 0.20 < x ≤ 1.0 are characterized by an additional suppression of a glasslike thermal conductivity in the temperature interval T_{N} < T < T* and a change in the slope of 1/χ(T). We argue that T* represents a temperature below which spin and orbital fluctuations couple together via λL∙S.
NASA Astrophysics Data System (ADS)
Cheng, Lan; Gauss, Jürgen
2011-06-01
We report an analytical scheme for the calculation of first-order electrical properties using the spin-free Dirac-Coulomb (SFDC) Hamiltonian, thereby exploiting the well-developed density-matrix formulations in nonrelativistic coupled-cluster (CC) derivative theory. Orbital relaxation effects are fully accounted for by including the relaxation of the correlated orbitals with respect to orbitals of all types, viz., frozen-core, occupied, virtual, and negative energy state orbitals. To demonstrate the applicability of the presented scheme, we report benchmark calculations for first-order electrical properties of the hydrogen halides, HX with X = F, Cl, Br, I, At, and a first application to the iodo(fluoro)methanes, CHnF3 - nI, n = 0-3. The results obtained from the SFDC calculations are compared to those from nonrelativistic calculations, those obtained via leading-order direct perturbation theory as well as those from full Dirac-Coulomb calculations. It is shown that the full inclusion of spin-free (SF) relativistic effects is necessary to obtain accurate first-order electrical properties in the presence of fifth-row elements. The SFDC scheme is also recommended for applications to systems containing lighter elements because it introduces no extra cost in the rate-determining steps of a CC calculation in comparison to the nonrelativistic case. On the other hand, spin-orbit contributions are generally small for first-order electrical properties of closed-shell molecules and may be handled efficiently by means of perturbation theory.
NASA Astrophysics Data System (ADS)
Bozkaya, Uǧur
2011-12-01
In this research, orbital-optimized third-order Møller-Plesset perturbation theory (OMP3) and its spin-component and spin-opposite scaled variants (SCS-OMP3 and SOS-OMP3) are introduced. Using a Lagrangian-based approach, an efficient, quadratically convergent algorithm for variational optimization of the molecular orbitals (MOs) for third-order Møller-Plesset perturbation theory (MP3) is presented. Explicit equations for response density matrices, the MO gradient, and Hessian are reported in spin-orbital form. The OMP3, SCS-OMP3, and SOS-OMP3 approaches are compared with the second-order Møller-Plesset perturbation theory (MP2), MP3, coupled-cluster doubles (CCD), optimized-doubles (OD), and coupled-cluster singles and doubles (CCSD) methods. All these methods are applied to the O4 +, O3, and seven diatomic molecules. Results demonstrate that the OMP3 and its variants provide significantly better vibrational frequencies than MP3, CCSD, and OD for the molecules where the symmetry-breaking problems are observed. For O4 +, the OMP3 prediction, 1343 cm-1, for ω6 (b3u) mode, where symmetry-breaking appears, is even better than presumably more reliable methods such as Brueckner doubles (BD), 1194 cm-1, and OD, 1193 cm-1, methods (the experimental value is 1320 cm-1). For O3, the predictions of SCS-OMP3 (1143 cm-1) and SOS-OMP3 (1165 cm-1) are remarkably better than the more robust OD method (1282 cm-1); the experimental value is 1089 cm-1. For the seven diatomics, again the SCS-OMP3 and SOS-OMP3 methods provide the lowest average errors, |Δωe| = 44 and |Δωe| = 35 cm-1, respectively, while for OD, |Δωe| = 161 cm-1and CCSD |Δωe| = 106 cm-1. Hence, the OMP3 and especially its spin-scaled variants perform much better than the MP3, CCSD, and more robust OD approaches for considered test cases. Therefore, considering both the computational cost and the reliability, SCS-OMP3 and SOS-OMP3 appear to be the best methods for the symmetry-breaking cases, based on
Magnetic damping and spin polarization of highly ordered B2 Co{sub 2}FeAl thin films
Cui, Yishen; Lu, Jiwei; Schäfer, Sebastian; Khodadadi, Behrouz; Mewes, Tim; Osofsky, Mike; Wolf, Stuart A.
2014-08-21
Epitaxial Co{sub 2}FeAl films were synthesized using the Biased Target Ion Beam Deposition technique. Post annealing yielded Co{sub 2}FeAl films with an improved B2 chemical ordering. Both the magnetization and the Gilbert damping parameter were reduced with increased B2 ordering. A low damping parameter, ∼0.002, was attained in B2 ordered Co{sub 2}FeAl films without the presence of the L2{sub 1} Heusler phase, which suggests that the B2 structure is sufficient for providing low damping in Co{sub 2}FeAl. The spin polarization was ∼53% and was insensitive to the chemical ordering.
NASA Technical Reports Server (NTRS)
Uemura, Y. J.; Kossler, W. J.; Kempton, J. R.; Yu, X. H.; Schone, H. E.; Opie, D.; Stronach, C. E.; Brewer, J. H.; Kiefl, R. F.; Kreitzman, S. R.
1988-01-01
Muon spin rotation and neutron scattering studies on powder and single-crystal specimens of La2CuO(4-y) are compared. The apparent difference between the muon and neutron results for the ordered moment in the antiferromagnetic state is interpreted as the signature of increasingly short-ranged spatial spin correlations with increasing oxygen content.
Glass-like recovery of antiferromagnetic spin ordering in a photo-excited manganite Pr0.7Ca0.3MnO3
Zhou, S.Y.; Langner, M.C.; Zhu, Y.; Chuang, Y.-D.; Rini, M.; Glover, T.E.; Hertlein, M.P.; Gonzalez, A.G. Cruz; Tahir, N.; Tomioka, Y.; Tokura, Y.; Hussain, Z.; Schoenlein, R.W.
2014-01-16
Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr0:7Ca0:3MnO3 following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.
Draeger, Guenter; Machek, Pavel
2003-01-24
We report the first experimental spin projections of empty partial density of states in antiferromagnetic NiO and CuO, paramagnetic MnO and in ferrimagnetic Dy3Fe5O12 by means of resonant X-ray scattering (RXS). Resolving resonantly scattered K{alpha}1,2 , K{beta}1,3 , L{alpha}1 and L1 core line spectra into their spin-up and spin-down components the spin character of the dipole- and quadrupole-excited conduction band states can quantitatively be analyzed. Since the method employs spin conservation in the RXS process and local spin references, it needs neither circularly polarized radiation nor sample magnetization for measuring the spectra. Hence, antiferro- and paramagnetic materials can be investigated as well. In the paper, the basic idea of the novel method, its experimental realization and the data treatment are reported including the spectra decomposition into the spin-up and spin-down components by using Principal Component Analysis (PCA). New and unambiguous results will be presented providing the opportunity to verify experimentally the results of spin-dependent (LSDA+U) calculations. So we argue the new spectroscopy complements X-ray magnetic dichroism, which is silent for antiferro- and paramagnetic materials. In fact, the novel method gives insight into the spin polarization of conduction band states in correlated materials, independently on their magnetic ordering.
Grabowski, Ireneusz Śmiga, Szymon; Buksztel, Adam; Fabiano, Eduardo; Teale, Andrew M.; Sala, Fabio Della
2014-07-14
The performance of correlated optimized effective potential (OEP) functionals based on the spin-resolved second-order correlation energy is analysed. The relative importance of singly- and doubly- excited contributions as well as the effect of scaling the same- and opposite- spin components is investigated in detail comparing OEP results with Kohn–Sham (KS) quantities determined via an inversion procedure using accurate ab initio electronic densities. Special attention is dedicated in particular to the recently proposed scaled-opposite–spin OEP functional [I. Grabowski, E. Fabiano, and F. Della Sala, Phys. Rev. B 87, 075103 (2013)] which is the most advantageous from a computational point of view. We find that for high accuracy, a careful, system dependent, selection of the scaling coefficient is required. We analyse several size-extensive approaches for this selection. Finally, we find that a composite approach, named OEP2-SOSh, based on a post-SCF rescaling of the correlation energy can yield high accuracy for many properties, being comparable with the most accurate OEP procedures previously reported in the literature but at substantially reduced computational effort.
NASA Astrophysics Data System (ADS)
Huang, Cheng-Yi; Lin, Hsin; Wang, Yung Jui; Bansil, Arun; Tsai, Wei-Feng
2016-05-01
We have investigated spin reorientation phenomena and interaction-driven effects under the presence of applied strains on the (001) surface of Pb1 -xSnx (Te, Se) topological crystalline insulators, which host multiple Dirac cones. Our analysis is based on a four-band k .p model, which captures the spin and orbital textures of the surface states at low energies around the X ¯ and Y ¯ points, including the Lifshitz transition. Even without breaking the time-reversal symmetry, we find that certain strains that break the mirror symmetry can induce a hedgehoglike spin texture associated with gap formation at the Dirac points. The Chern number of the gapped surface ground state is shown to be tunable through the interplay of strains and a perpendicular Zeeman field. We also consider the effects of strain in the presence of interactions in driving competing orders, and we obtain the associated phase diagram at the mean-field level. Potential applications of our results for low power consuming electronics are discussed.
Charge and Spin Ordering in Insulator Na0.5CoO2: Effects of Correlation and Symmetry
NASA Astrophysics Data System (ADS)
Lee, Kwan-Woo; Pickett, Warren
2006-03-01
The discovery by Takada and coworkers of superconductivity in Na0.3CoO21.3 H2O near 5K has led to extensive studies of the rich variation of properties in the NaxCoO2 system (0.2 <=x <=1), which has a triangular lattice of Co sites and a layered structure. In addition, specifically at x=0.5, the system has been observed to undergo a charge disproportionation (2Co^3.5+ -> Co^3++Co^4+) and metal-insulator transition at 50 K, while the rest of the phase diagram is metallic. We will present results of studies of charge disproportionation and charge- and spin-ordering in insulating in Na0.5CoO2, applying ab initio band theory including correlations due to intra-atomic repulsion. Various ordering patterns (zigzag and two striped) for four-Co supercells are analyzed before focusing on the observed ``out-of-phase stripe'' pattern of antiferromagnetic Co^4+ spins along charge-ordered stripes. This pattern relieves frustration and shows distinct analogies with the cuprate layers: a bipartite lattice of antialigned spins, with axes at 90^o angles. Substantial distinctions with cuprates are also discussed, including the tiny gap of a new variant of ``charge transfer'' type within the Co 3d system. [References] [1] K. Takada et al., Nature 422, 53 (2003). [2] M. L. Foo et al., Phys. Rev. Lett. 92,247001 (2004). [3] K.-W. Lee, J. Kunes, P. Novak, and W. E. Pickett, Phys. Rev. Lett. 94, 026403 (2005). [4] K.-W. Lee and W. E. Pickett, cond-mat/0510555.
Magnetic order in α -RuCl3 : A honeycomb-lattice quantum magnet with strong spin-orbit coupling
NASA Astrophysics Data System (ADS)
Sears, J. A.; Songvilay, M.; Plumb, K. W.; Clancy, J. P.; Qiu, Y.; Zhao, Y.; Parshall, D.; Kim, Young-June
2015-04-01
We report magnetic and thermodynamic properties of single crystal α -RuCl3 , in which the Ru3+(4 d5) ion is in its low spin state and forms a honeycomb lattice. Two features are observed in both magnetic susceptibility and specific heat data; a sharp peak at 7 K and a broad hump near 10-15 K. In addition, we observe a metamagnetic transition between 5 and 10 T. Our neutron diffraction study of single crystal samples confirms that the low temperature peak in the specific heat is associated with a magnetic order with unit cell doubling along the honeycomb (100) direction, which is consistent with zigzag order, one of the types of magnetic order predicted within the framework of the Kitaev-Heisenberg model.
Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2O7
NASA Astrophysics Data System (ADS)
Castellano, C.; Berti, G.; Sanna, S.; Ruiz-Bustos, R.; van Duijn, J.; Brambilla, A.; Muñoz-Noval, Á.; Carretta, P.; Duò, L.; Demartin, F.
2015-06-01
We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Néel temperature TN˜77 K pointed out by a huge Debye-Waller σ2 factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T*=150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.
Gaffney, B J; Marsh, D
1998-10-27
The EPR spectra of spin-labeled lipid chains in fully hydrated bilayer membranes of dimyristoyl phosphatidylcholine containing 40 mol % of cholesterol have been studied in the liquid-ordered phase at a microwave radiation frequency of 94 GHz. At such high field strengths, the spectra should be optimally sensitive to lateral chain ordering that is expected in the formation of in-plane domains. The high-field EPR spectra from random dispersions of the cholesterol-containing membranes display very little axial averaging of the nitroxide g-tensor anisotropy for lipids spin labeled toward the carboxyl end of the sn-2 chain (down to the 8-C atom). For these positions of labeling, anisotropic 14N-hyperfine splittings are resolved in the gzz and gyy regions of the nonaxial EPR spectra. For positions of labeling further down the lipid chain, toward the terminal methyl group, the axial averaging of the spectral features systematically increases and is complete at the 14-C atom position. Concomitantly, the time-averaged
NASA Astrophysics Data System (ADS)
Takashima, Hirokazu; Ishihara, Sumio
2010-03-01
In order to study for novel spin and charge orders in strongly correlated electron systems in frustrated lattices,we investigated extended Hubbard model in 2 dimensional (2D) checkerboard and triangular lattices using the functional renormalization group method(fRG) with an improved algorithm [1]. In this method, both the quantum effect and the geometrical frustration effect at finite temperature are taken into account properly. Non-monotonic temperature dependence of the spin susceptibility was observed both in the models . In a 2D isotropic triangular lattice at half-filling, divergence of the particle-particle channel vertex functions was observed in a region of the intermediate value of the on-site Coulomb interaction. We have also investigated the extended Hubbard model with long-range Coulomb interactions. A possibility of the ferromagnetic order and calculations with including the self-energy correction will be introduced .[1] H. Takashima, R. Arita, K. Kuroki, and H. Aoki, J. Phys.: Conf. Ser, 150, 052261 (2009)
Long-range magnetic order and spin-lattice coupling in delafossite CuFeO2
NASA Astrophysics Data System (ADS)
Eyert, Volker; Frésard, Raymond; Maignan, Antoine
2008-08-01
The electronic and magnetic properties of the delafossite CuFeO2 are investigated by means of electronic structure calculations. They are performed using density functional theory in the generalized gradient approximation, as well as the new full-potential augmented spherical wave method. The calculations reveal three different spin states at the iron sites. Using for the first time the experimentally determined low-temperature crystal structure, we find long-range antiferromagnetic ordering in agreement with experiment. In addition, our calculations show that nonlocal interactions as covered by the generalized gradient approximation lead to a semiconducting ground state.
Tuning Effects of Spin-Orbit Coupling in L10 Ordered and Disordered FePdPt Films
NASA Astrophysics Data System (ADS)
Fan, W. J.; Shi, Z.; Chen, F. L.; Zhou, S. M.
2015-09-01
Effects of spin-orbit coupling (SOC) on magnetocrystalline anisotropy, magneto-optical Kerr effect (MOKE), magnetic damping parameter and anomalous Hall effect (AHE) have been studied in theory extensively. In contrast, few experimental reports have appeared on these issues. In this review paper, we introduce our recent experimental investigation on the SOC tuning effects on the perpendicular magnetic anisotropy, polar MOKE, intrinsic magnetic damping parameter and AHE in L10 ordered Fe0.5(Pd1-xPtx)0.5 ternary alloys. We also outline the SOC effects in polycrystalline disordered Fe0.5(Pd1-xPtx)0.5 films for comparison.
Magnetic orders and spin-flop transitions in the cobalt doped multiferroic $\\rm Mn_{1-x}Co_{x}WO_4$
Chi, Songxue; Fernandez-Baca, Jaime A; Cao, Huibo; Liang, K. C.; Wang, Y. Q.; Lorenz, Bernd; Chu, C. W.
2012-01-01
We present a comprehensive single crystal neutron diffraction investigation of the $\\rm Mn_{1-x}Co_{x}WO_4$ with $0.02\\leq x \\leq0.30$. At lower concentration $x \\leq 0.05$, the system is quickly driven into the multiferroic phase with spin structure forming an elliptical spiral order similar to the parent compound. The reduction of electric polarization is ascribed to the tilting of the spiral plane. For $x\\sim 0.075$, the magnetic structure undergoes a spin flop transition that is characterized by a sudden rotation of the spin helix envelope into the $ac$ plane. This spin structure persists for concentration up to $x=0.15$, where additional competing magnetic orders appear at low temperature. For $0.17 \\leq x \\leq 0.30$, the system experiences another spin flop transition and recovers the low-$x$ spiral spin configuration. A simple commensurate spin structure with $\\vec{q}=(0.5,0,0)$ is found to coexist with the incommensurate spiral order. The complex evolution of magnetic structure in Co doped $\\rm MnWO_4$ contrasts sharply with other transition metal ion doped $\\rm Mn_{1-x}A_xWO_4$ (A=Zn, Mg, Fe) where the chemical substitutions stabilize only one type of magnetic structure. The rich phase diagram of $\\rm Mn_{1-x}Co_{x}WO_4 $ results from the interplay between magnetic frustration and spin anisotropy of the Co ions.
NASA Astrophysics Data System (ADS)
Bohé, Alejandro; Faye, Guillaume; Marsat, Sylvain; Porter, Edward K.
2015-10-01
We investigate the dynamics of spinning binaries of compact objects at the next-to-leading order in the quadratic-in-spin effects, which corresponds to the third post-Newtonian order (3PN). Using a Dixon-type multipolar formalism for spinning point particles endowed with spin-induced quadrupoles and computing iteratively in harmonic coordinates the relevant pieces of the PN metric within the near zone, we derive the post-Newtonian equations of motion as well as the equations of spin precession. We find full equivalence with available results. We then focus on the far-zone field produced by those systems and obtain the previously unknown 3PN spin contributions to the gravitational-wave energy flux by means of the multipolar post-Minkowskian wave generation formalism. Our results are presented in the center-of-mass frame for generic orbits, before being further specialized to the case of spin-aligned, circular orbits. Based on the energy balance equation, we derive the orbital phase of the binary at the order 3PN including all conservative spin effects and briefly discuss the relevance of the new terms.
NASA Astrophysics Data System (ADS)
Raghuvanshi, Nimisha; Singh, Avinash
2010-10-01
Spin waves in the (0, π) and (0, π, π) ordered spin-density-wave (SDW) states of the t-t' Hubbard model are investigated at finite doping. In the presence of small t', these composite ferro-antiferromagnetic (F-AF) states are found to be strongly stabilized at finite hole doping due to enhanced carrier-induced ferromagnetic spin couplings as in metallic ferromagnets. Anisotropic spin-wave velocities, a spin-wave energy scale of around 200 meV, reduced magnetic moment and rapid suppression of magnetic order with electron doping x (corresponding to F substitution of O atoms in LaO1 - xFxFeAs or Ni substitution of Fe atoms in BaFe2 - xNixAs2) obtained in this model are in agreement with observed magnetic properties of doped iron pnictides.
Field-controlled spin-density-wave order and quantum critically in Sr3 Ru2 O7
NASA Astrophysics Data System (ADS)
Hayden, Stephen
The quasi-2D metamagnetic perovskite metal Sr3Ru2O7 has been an enigma for the last decade. The application of a large magnetic field of 8T parallel to the c-axis creates a new phase at low temperatures. This phase shows ``electronic nematic'' properties in that strong anisotropy its resistivity can be created by tilting the field away from the c-axis. In addition, measurement of transport and thermodynamic properties suggest that the phase is at the centre of a quantum critical region. Here we use neutron scattering to show that the magnetic field actually induces spin-density-wave magnetic order in the proximity of a metamagnetic critical endpoint. In fact, Sr3Ru2O7 can be tuned through two magnetically-ordered SDW states which exist over relatively small ranges in field (< 0.4 T). Their origin is probably due to the electronic fine structure near the Fermi energy. The magnetic field direction is shown to control the SDW domain populations which naturally explains the strong resistivity anisotropy or ''electronic nematic'' behaviour observed in this material. We find that Sr3Ru2O7 is also unique in that its the quantum critical region is controlled by overdamped incommensurate low-energy spin fluctuations with a diverging relaxation time. The low-energy electronic properties reflect the presence of these fluctuations and, in particular, the field-dependent low-temperature specific heat is proportional to the spin relaxation rate. [Based on C. Lester, S. Ramos, R. S. Perry at el. Natural Materials 14, 373 (2015).
Zhang, Qiang; Fernandes, Rafael M.; Lamsal, Jagat; Yan, Jiaqiang; Chi, Songxue; Tucker, Gregory S.; Pratt, Daniel K.; Lynn, Jeffrey W.; McCallum, R. W.; Canfield, Paul C.; et al
2015-02-04
Inelastic neutron scattering is employed to investigate the impact of electronic nematic order on the magnetic spectra of LaFeAsO and Ba(Fe0.953Co0.047)2As2. These materials are ideal to study the paramagnetic-nematic state, since the nematic order, signaled by the tetragonal-to-orthorhombic transition at TS, sets in well above the stripe antiferromagnetic ordering at TN. We find that the temperature-dependent dynamic susceptibility displays an anomaly at TS followed by a sharp enhancement in the spin-spin correlation length, revealing a strong feedback effect of nematic order on the low-energy magnetic spectrum. As a result, our findings can be consistently described by a model that attributesmore » the structural or nematic transition to magnetic fluctuations, and unveils the key role played by nematic order in promoting the long-range stripe antiferromagnetic order in iron pnictides.« less
ELASTIC MEMBRANE DEFORMATIONS GOVERN INTERLEAFLET COUPLING OF LIPID-ORDERED DOMAINS
Galimzyanov, Timur R.; Molotkovsky, Rodion J.; Bozdaganyan, Marine E.; Cohen, Fredric S.; Pohl, Peter; Akimov, Sergey A.
2016-01-01
The mechanism responsible for domain registration in two membrane leaflets has thus far remained enigmatic. Using continuum elasticity theory, we show that minimum line tension is achieved along the rim between thicker (ordered) and thinner (disordered) domains by shifting the rims in opposing leaflets by a few nanometers relative to each other. Increasing surface tension yields an increase in line tension, resulting in larger domains. Because domain registration is driven by lipid deformation energy, it does not require special lipid components nor interactions at the membrane midplane. PMID:26340212
Elastic Membrane Deformations Govern Interleaflet Coupling of Lipid-Ordered Domains.
Galimzyanov, Timur R; Molotkovsky, Rodion J; Bozdaganyan, Marine E; Cohen, Fredric S; Pohl, Peter; Akimov, Sergey A
2015-08-21
The mechanism responsible for domain registration in two membrane leaflets has thus far remained enigmatic. Using continuum elasticity theory, we show that minimum line tension is achieved along the rim between thicker (ordered) and thinner (disordered) domains by shifting the rims in opposing leaflets by a few nanometers relative to each other. Increasing surface tension yields an increase in line tension, resulting in larger domains. Because domain registration is driven by lipid deformation energy, it does not require special lipid components or interactions at the membrane midplane. PMID:26340212
Ferromagnetic ordered phase of quantum spin ice system Yb2Ti2O7 under [001] magnetic field
NASA Astrophysics Data System (ADS)
Hamachi, Noriaki; Yasui, Yukio; Araki, Koji; Kittaka, Shunichiro; Sakakibara, Toshiro
2016-05-01
Measurements of magnetization (M) and specific heat (C) under a [001] magnetic field were carried out on a single crystal of a quantum spin ice system Yb2Ti2O7 in order to investigate a feature of the transition occurred at TC ˜ 0.2 K. As a result of applying the magnetic field μ0H < 0.1 T, the C/T - T curve structure and transition temperature barely changed. On the other hand, applying the more than 0.1 T magnetic field, the C/T - T curve structure drastically change from sharp peak structure to broad peak one, and the broad peak temperature of C/T - T curves linearly increases with increasing magnetic field (H). In the magnetic field μ0H < 0.1 T, the magnetization drastically increases around TC ˜ 0.2 K with decreasing T, and a thermal hysteresis loop of the M - T curve is observed. With increasing H, the thermal hysteresis loop of the M - T curves disappears above μ0HC = 0.1 T. We can understand these results, where Yb2Ti2O7 exhibits a first-order ferromagnetic transition associated with the latent heat corresponding to the energy of μ0HC = 0.1 T. Basis of the H - T phase diagram along [001] magnetic field, the feature of the transition occurred at TC ˜ 0.2 K in quantum spin ice system Yb2Ti2O7 is discussed.
Magnetic ordering and spin-reorientation transitions in TbCo{sub 3}B{sub 2}
Dubman, Moshe; Caspi, El'ad N.; Ettedgui, Hanania; Keller, Lukas; Melamud, Mordechai; Shaked, Hagai
2005-07-01
The magnetic structure of the compound TbCo{sub 3}B{sub 2} has been studied in the temperature range 1.5 K{<=}T{<=}300 K by means of neutron powder diffraction, magnetization, magnetic ac susceptibility, and heat capacity measurements. The compound is of hexagonal symmetry and is paramagnetic at 300 K, undergoes a magnetic Co-Co ordering transition at {approx}170 K, and a second magnetic Tb-Tb ordering transition at {approx}30 K. The latter induces a spin-reorientation transition, in which the magnetic axis rotates from the c axis toward the basal plane. Below this transition a symmetry decrease ({gamma} magnetostriction) sets in, leading to an orthorhombic distortion of the crystal lattice. The crystal and magnetic structures and interactions and their evolution with temperature are discussed using a microscopic physical model.
Comment on "Elastic Membrane Deformations Govern Interleaflet Coupling of Lipid-Ordered Domains"
NASA Astrophysics Data System (ADS)
Williamson, J. J.; Olmsted, P. D.
2016-02-01
In lieu of abstract, first paragraph reads: Galimzyanov et al. [1] find that line tension between thick liquid-ordered ($L_{o}$) and thinner liquid-disordered ($L_{d}$) registered lipid bilayer phases is minimised by an asymmetric "slip region", length $L\\!\\sim\\!5\\,\\textrm{nm}$ (Fig. 1). They claim that line tensions alone explain domain registration, without "direct" (area-dependent) inter-leaflet interaction [2,3]. We show this is unfounded, without direct interaction their results would predict \\textit{antiregistration}, dependent on composition. To find equilibrium from line energies, line \\textit{tensions} must be combined with interfacial lengths for given states at given composition. This was not done in [1].
Adaptive rheology and ordering of cell cytoskeleton govern matrix rigidity sensing
Gupta, Mukund; Sarangi, Bibhu Ranjan; Deschamps, Joran; Nematbakhsh, Yasaman; Callan-Jones, Andrew; Margadant, Felix; Mège, René-Marc; Lim, Chwee Teck; Voituriez, Raphaël; Ladoux, Benoît
2015-01-01
Matrix rigidity sensing regulates a large variety of cellular processes and has important implications for tissue development and disease. However, how cells probe matrix rigidity, and hence respond to it, remains unclear. Here, we show that rigidity sensing and adaptation emerge naturally from actin cytoskeleton remodeling. Our in vitro experiments and theoretical modeling demonstrate a bi-phasic rheology of the actin cytoskeleton, which transitions from fluid on soft substrates to solid on stiffer ones. Furthermore, we find that increasing substrate stiffness correlates with the emergence of an orientational order in actin stress fibers, which exhibit an isotropic to nematic transition that we characterize quantitatively in the framework of active matter theory. These findings imply mechanisms mediated by a large-scale reinforcement of actin structures under stress, which could be the mechanical drivers of substrate stiffness dependent cell shape changes and cell polarity. PMID:26109233
Investigation of spin ordering in antiferromagnetic Fe1-xMnxPO4 with Mössbauer spectroscopy
NASA Astrophysics Data System (ADS)
Jun Kwon, Woo; Wha Lee, Bo; Sung Kim, Chul
2013-05-01
We have investigated the spin ordering in Fe1-xMnxPO4, which is a possible cathode material for rechargeable lithium ion battery, with antiferromagnetic structure below Néel temperature (TN). The prepared Fe1-xMnxPO4 (x = 0.0, 0.1, and 0.3) samples have orthorhombic structures with space group of Pnma. These samples show the magnetic phase transition, caused by the strong crystalline field at the MO6 octahedral sites. According to the temperature dependence of magnetic susceptibility of Fe1-xMnxPO4, all samples show antiferromagnetic behaviors. The Néel temperature (TN) decreases from 114 K at x = 0.0 to 97 K at x = 0.3 with Mn concentrations. The magnetization of Fe1-xMnxPO4 decreases until the temperature reaches the spin-reorientation (TS) temperature, and then starts increasing as the temperature increases up to TN. The TS of the Fe1-xMnxPO4 were found to be 30, 27, and 24 K for x = 0.0, 0.1, and 0.3. In order to investigate the hyperfine interaction of Fe3+ ions in FeO6 octahedral sites, Mössbauer spectra of Fe1-xMnxPO4 have been taken at various temperatures from 4.2 to 295 K. The isomer shift (δ) values of the Fe1-xMnxPO4 were between 0.31 and 0.43 mm/s, indicating the high spin state of Fe3+ at all temperatures. The magnetic hyperfine field (Hhf) and electric quadrupole splitting (ΔEQ) values of Fe0.9Mn0.1PO4 at 4.2 K were determined to be Hhf = 498 kOe and ΔEQ = 2.1 mm/s. We have also observed the abrupt changes in Hhf and ΔEQ at 27 K for Fe0.9Mn0.1PO4, and decrease the value of TS of Fe1-xMnxPO4 with Mn concentrations. Our study suggests that these changes in Fe1-xMnxPO4 are originated from the strong electric crystalline field and spin-orbit coupling of FeO6 octahedral site.
NMR probing of spin and charge order near odd-integer filling in the second Landau level
NASA Astrophysics Data System (ADS)
Rhone, T. D.; Tiemann, L.; Muraki, K.
2015-07-01
Studies of spin degrees of freedom near odd-integer filling ν =3 in the second Landau level have engendered conflicting accounts of the spin properties in this regime. Using resistively detected NMR as a probe of local spin density, we explore the nature of the ground state in the quantum Hall regime near ν =3 . Our Knight shift measurements reveal anomalies in NMR spectral line shapes near ν =3 , which demonstrate the presence of solid phases formed from charged quasiparticles, with maximal spin polarization (i.e., no additional spin flips) at each ν . The long nuclear spin relaxation times demonstrate the absence of Skyrmions, or spin textures, in this phase. On the basis of these observations, we attempt to reconcile conflicting reports on the quasiparticle properties and spin wave excitations at ν ˜3 , which may engender new paradigms for the understanding of spin excitations in a collinear ferromagnet with broken translational symmetry.
Maurice, Rémi; Réal, Florent; Gomes, André Severo Pereira; Vallet, Valérie; Montavon, Gilles; Galland, Nicolas
2015-03-01
The nature of chemical bonds in heavy main-group diatomics is discussed from the viewpoint of effective bond orders, which are computed from spin-orbit wave functions resulting from spin-orbit configuration interaction calculations. The reliability of the relativistic correlated wave functions obtained in such two-step spin-orbit coupling frameworks is assessed by benchmark studies of the spectroscopic constants with respect to either experimental data, or state-of-the-art fully relativistic correlated calculations. The I2, At2, IO(+), and AtO(+) species are considered, and differences and similarities between the astatine and iodine elements are highlighted. In particular, we demonstrate that spin-orbit coupling weakens the covalent character of the bond in At2 even more than electron correlation, making the consideration of spin-orbit coupling compulsory for discussing chemical bonding in heavy (6p) main group element systems. PMID:25747079
NASA Astrophysics Data System (ADS)
Maurice, Rémi; Réal, Florent; Gomes, André Severo Pereira; Vallet, Valérie; Montavon, Gilles; Galland, Nicolas
2015-03-01
The nature of chemical bonds in heavy main-group diatomics is discussed from the viewpoint of effective bond orders, which are computed from spin-orbit wave functions resulting from spin-orbit configuration interaction calculations. The reliability of the relativistic correlated wave functions obtained in such two-step spin-orbit coupling frameworks is assessed by benchmark studies of the spectroscopic constants with respect to either experimental data, or state-of-the-art fully relativistic correlated calculations. The I2, At2, IO+, and AtO+ species are considered, and differences and similarities between the astatine and iodine elements are highlighted. In particular, we demonstrate that spin-orbit coupling weakens the covalent character of the bond in At2 even more than electron correlation, making the consideration of spin-orbit coupling compulsory for discussing chemical bonding in heavy (6p) main group element systems.
Stan, Raluca-Maria; Gaina, Roxana; Enachescu, Cristian E-mail: radu.tanasa@uaic.ro; Stancu, Alexandru; Tanasa, Radu E-mail: radu.tanasa@uaic.ro; Bronisz, Robert
2015-05-07
In this paper, we analyze two types of hysteresis in spin crossover molecular magnets compounds in the framework of the First Order Reversal Curve (FORC) method. The switching between the two stable states in these compounds is accompanied by hysteresis phenomena if the intermolecular interactions are higher than a threshold. We have measured the static thermal hysteresis (TH) and the kinetic light induced thermal hysteresis (LITH) major loops and FORCs for the polycrystalline Fe(II) spin crossover compound [Fe{sub 1−x}Zn{sub x}(bbtr){sub 3}](ClO{sub 4}){sub 2} (bbtr = 1,4-di(1,2,3-triazol-1-yl)butane), either in a pure state (x = 0) or doped with Zn ions (x = 0.33) considering different sweeping rates. Here, we use this method not only to infer the domains distribution but also to disentangle between kinetic and static components of the LITH and to estimate the changes in the intermolecular interactions introduced by dopants. We also determined the qualitative relationship between FORC distributions measured for TH and LITH.
NASA Astrophysics Data System (ADS)
Wang, Yuxuan; Cho, Gil Young; Hughes, Taylor L.; Fradkin, Eduardo
2016-04-01
We analyze the superconducting instabilities in the vicinity of the quantum-critical point of an inversion symmetry breaking order. We first show that the fluctuations of the inversion symmetry breaking order lead to two degenerate superconducting (SC) instabilities, one in the s -wave channel, and the other in a time-reversal invariant odd-parity pairing channel (the simplest case being the same as the of 3He-B phase). Remarkably, we find that unlike many well-known examples, the selection of the pairing symmetry of the condensate is independent of the momentum-space structure of the collective mode that mediates the pairing interaction. We found that this degeneracy is a result of the existence of a conserved fermionic helicity χ , and the two degenerate channels correspond to even and odd combinations of SC order parameters with χ =±1 . As a result, the system has an enlarged symmetry U (1 ) ×U (1 ) , with each U (1 ) corresponding to one value of the helicity χ . Because of the enlarged symmetry, this system admits exotic topological defects such as a fractional quantum vortex, which we show has a Majorana zero mode bound at its core. We discuss how the enlarged symmetry can be lifted by small perturbations, such as the Coulomb interaction or Fermi surface splitting in the presence of broken inversion symmetry, and we show that the resulting superconducting state can be topological or trivial depending on parameters. The U (1 ) ×U (1 ) symmetry is restored at the phase boundary between the topological and trivial SC states, and allows for a transition between topologically distinct SC phases without the vanishing of the order parameter. We present a global phase diagram of the superconducting states and discuss possible experimental implications.
NASA Astrophysics Data System (ADS)
Levchenko, A.; Vavilov, M. G.; Khodas, M.; Chubukov, A. V.
2013-04-01
Recent measurements of the doping dependence of the London penetration depth λ(x) at low T in clean samples of isovalent BaFe2(As1-xPx)2 at T≪Tc [Hashimoto et al., Science 336, 1554 (2012)SCIEAS0036-8075] revealed a peak in λ(x) near optimal doping x=0.3. The observation of the peak at T≪Tc, points to the existence of a quantum critical point beneath the superconducting dome. We associate such a quantum critical point with the onset of a spin-density-wave order and show that the renormalization of λ(x) by critical magnetic fluctuations gives rise to the observed feature. We argue that the case of pnictides is conceptually different from a one-component Galilean invariant Fermi liquid, for which correlation effects do not cause the renormalization of the London penetration depth at T=0.
Collinear spin-density-wave ordering in Fe/Cr multilayers and wedges
Fishman, R.S.; Shi, Z.
1999-06-01
Several recent experiments have detected a spin-density wave (SDW) within the Cr spacer of Fe/Cr multilayers and wedges. We use two simple models to predict the behavior of a collinear SDW within an Fe/Cr/Fe trilayer. Both models combine assumed boundary conditions at the Fe-Cr interfaces with the free energy of the Cr spacer. Depending on the temperature and the number {ital N} of Cr monolayers, the SDW may be either commensurate ({ital C}) or incommensurate ({ital I}) with the bcc Cr lattice. Model I assumes that the Fe-Cr interface is perfect and that the Fe-Cr interaction is antiferromagnetic. Consequently, the {ital I} SDW antinodes lie near the Fe-Cr interfaces. With increasing temperature, the Cr spacer undergoes a series of transitions between {ital I} SDW phases with different numbers {ital n} of nodes. If the {ital I} SDW has n=m nodes at T=0, then {ital n} increases by one at each phase transition from {ital m} to m{minus}1 to m{minus}2 up to the {ital C} phase with n=0 above T{sub IC}(N). For a fixed temperature, the magnetic coupling across the Cr spacer undergoes a phase slip whenever {ital n} changes by one. In the limit N{r_arrow}{infinity}, T{sub IC}(N) is independent of the Fe-Cr coupling strength. We find that T{sub IC}({infinity}) is always larger than the bulk N{acute e}el transition temperature and increases with the strain on the Cr spacer. These results explain the very high IC transition temperature of about 600 K extrapolated from measurements on Fe/Cr/Fe wedges. Model II assumes that the {ital I} SDW nodes lie precisely at the Fe-Cr interfaces. This condition may be enforced by the interfacial roughness of sputtered Fe/Cr multilayers. As a result, the {ital C} phase is never stable and the transition temperature T{sub N}(N) takes on a seesaw pattern as n{ge}2 increases with thickness. In agreement with measurements on both sputtered and epitaxially grown multilayers, model II predicts the {ital I} phase to be unstable above the bulk N
NASA Astrophysics Data System (ADS)
Ghosh, Pratyay; Verma, Akhilesh Kumar; Kumar, Brijesh
2016-01-01
A spin-1 Heisenberg model on trimerized kagome lattice is studied by doing a low-energy bosonic theory in terms of plaquette triplons defined on its triangular unit cells. The model considered has an intratriangle antiferromagnetic exchange interaction J (set to 1) and two intertriangle couplings J'>0 (nearest neighbor) and J″ (next nearest neighbor; of both signs). The triplon analysis performed on this model investigates the stability of the trimerized singlet ground state (which is exact in the absence of intertriangle couplings) in the J'-J″ plane. It gives a quantum phase diagram that has two gapless antiferromagnetically ordered phases separated by the spin-gapped trimerized singlet phase. The trimerized singlet ground state is found to be stable on J″=0 line (the nearest-neighbor case), and on both sides of it for J″≠0 , in an extended region bounded by the critical lines of transition to the gapless antiferromagnetic phases. The gapless phase in the negative J″ region has a coplanar 120∘ antiferromagnetic order with √{3 }×√{3 } structure. In this phase, all the magnetic moments are of equal length, and the angle between any two of them on a triangle is exactly 120∘. The magnetic lattice in this case has a unit cell consisting of three triangles. The other gapless phase, in the positive J″ region, is found to exhibit a different coplanar antiferromagnetic order with ordering wave vector q =(0 ,0 ) . Here, two magnetic moments in a triangle are of the same magnitude, but shorter than the third. While the angle between two short moments is 120∘-2 δ , it is 120∘+δ between a short and the long one. Only when J″=J' , their magnitudes become equal and the relative angles 120∘. The magnetic lattice in this q =(0 ,0 ) phase has the translational symmetry of the kagome lattice with triangular unit cells of reduced (isosceles) symmetry. This reduction in the point-group symmetry is found to show up as a difference in the intensities of
NASA Astrophysics Data System (ADS)
Kaul, S. N.; Messala, Umasankar
2016-03-01
Weak itinerant-electron ferromagnet Ni3Al is driven to magnetic instability (quantum critical point, QCP, where the long-range ferromagnetic order of the bulk ceases to exist) by reducing the average crystallite size to d=50 nm. 'Zero-field' (H=0) linear and nonlinear ac-susceptibilities, measured on Ni3Al nanoparticle aggregates, with d=50 nm (S1) and d=5 nm (S2), provide strong evidence for two spin glass (SG)-like thermodynamic phase transitions: one at Ti(H = 0) ≃ 30 K (Ti† (H = 0) ≃ 230 K) and the other at a lower temperature Tp(H = 0) ≃ 8 K (Th(H = 0) ≃ 52 K) in S1 (S2). 'In-field' (H ≠ 0) linear ac-susceptibility and dc magnetization demonstrate that the thermodynamic nature of these transitions is preserved in finite fields. The presently determined H-T phase diagrams for the samples S1 and S2 are compared with those predicted by the Kotliar-Sompolinsky and Gabay-Toulouse mean-field models and Monte Carlo simulations, based on the chirality-driven spin glass (SG) ordering scenario, for a three-dimensional nearest-neighbor Heisenberg SG system with or without weak random anisotropy. Such a detailed comparison permits us to unambiguously identify various 'zero-field' and 'in-field' SG phase transitions as: (i) the simultaneous paramagnetic (PM)-chiral glass (CG) and PM-SG phase transitions at Ti(H), (ii) the PM-CG transition at Ti† (H), (iii) the replica symmetry-breaking SG transition at Tp(H), and (iv) the continuous spin-rotation symmetry-breaking SG transition at Th(H). In the presence of random anisotropy, magnetization fails to saturate even at 90 kOe in S1 whereas negligibly small anisotropy allows even fields as weak as 1 kOe to saturate magnetization and induce ferromagnetism in S2. Due to the proximity to CG/SG-QCP, magnetization and susceptibility both exhibit non-Fermi liquid behavior over a wide range at low temperatures.
NASA Astrophysics Data System (ADS)
Ito, T. U.; Higemoto, W.; Sakai, A.; Tsujimoto, M.; Nakatsuji, S.
2015-09-01
The nature of multipolar order and hyperfine-enhanced (HE) 141Pr nuclear spin dynamics in PrV2Al20 was investigated using the muon spin relaxation technique. No explicit sign of time-reversal symmetry breaking was found below the multipolar order temperature TQ˜0.6 K in a zero applied field as anticipated on the basis of the antiferroquadrupolar (AFQ) order picture proposed by Sakai and Nakatsuji [J. Phys. Soc. Jpn. 80, 063701 (2011), 10.1143/JPSJ.80.063701]. Further evidence of the nonmagnetic ground state was obtained from the observation of HE 141Pr nuclear spin fluctuations in the MHz scale. A marked increase in the muon spin-lattice relaxation rate (1 /T1 ,μ) was observed below 1 K with decreasing temperature, which was attributed to the perturbation on the HE 141Pr nuclear spin dynamics associated with the development of AFQ correlations. The longitudinal field dependence of 1 /T1 ,μ revealed that the enhanced 141Pr nuclear spin accidentally has an effective gyromagnetic ratio close to that of the muon.
Jiang, Kun; Zhang, Yi; Zhou, Sen; Wang, Ziqiang
2015-05-29
We study the Hubbard model on the frustrated honeycomb lattice with nearest-neighbor hopping t_{1} and second nearest-neighbor hopping t_{2}, which is isomorphic to the bilayer triangle lattice, using the SU(2)-invariant slave boson theory. We show that the Coulomb interaction U induces antiferromagnetic (AF) chiral spin density wave (χSDW) order in a wide range of κ=t_{2}/t_{1} where both the two-sublattice AF order at small κ and the decoupled three-sublattice 120° order at large κ are strongly frustrated, leading to three distinct phases with different anomalous Hall responses. We find a continuous transition from a χSDW semimetal with the anomalous Hall effect to a topological chiral Chern insulator exhibiting the quantum anomalous Hall effect, followed by a discontinuous transition to a χSDW insulator with a zero total Chern number but an anomalous ac Hall effect. The χSDW is likely a generic phase of strongly correlated and highly frustrated hexagonal lattice electrons. PMID:26066448
NASA Astrophysics Data System (ADS)
Sadeghi, Azam; Alaei, Mojtaba; Shahbazi, Farhad; Gingras, Michel J. P.
2015-04-01
FeF3, with its half-filled Fe3 +3 d orbital, hence zero orbital angular momentum and S =5 /2 , is often put forward as a prototypical highly frustrated classical Heisenberg pyrochlore antiferromagnet. By employing ab initio density functional theory, we obtain an effective spin Hamiltonian for this material. This Hamiltonian contains nearest-neighbor antiferromagnetic Heisenberg, biquadratic, and Dzyaloshinskii-Moriya interactions as dominant terms and we use Monte Carlo simulations to investigate the nonzero temperature properties of this minimal model. We find that upon decreasing temperature, the system passes through a Coulomb phase, composed of short-range correlated coplanar states, before transforming into an "all-in/all-out" (AIAO) state via a very weakly first-order transition at a critical temperature Tc≈22 K, in good agreement with the experimental value for a reasonable set of Coulomb interaction U and Hund's coupling JH describing the material. Despite the transition being first order, the AIAO order parameter evolves below Tc with a power-law behavior characterized by a pseudo "critical exponent" β ≈0.18 in accord with experiment. We comment on the origin of this unusual β value.
NASA Astrophysics Data System (ADS)
Jiang, Kun; Zhang, Yi; Zhou, Sen; Wang, Ziqiang
2015-05-01
We study the Hubbard model on the frustrated honeycomb lattice with nearest-neighbor hopping t1 and second nearest-neighbor hopping t2, which is isomorphic to the bilayer triangle lattice, using the SU(2)-invariant slave boson theory. We show that the Coulomb interaction U induces antiferromagnetic (AF) chiral spin density wave (χ SDW ) order in a wide range of κ =t2/t1 where both the two-sublattice AF order at small κ and the decoupled three-sublattice 120° order at large κ are strongly frustrated, leading to three distinct phases with different anomalous Hall responses. We find a continuous transition from a χ SDW semimetal with the anomalous Hall effect to a topological chiral Chern insulator exhibiting the quantum anomalous Hall effect, followed by a discontinuous transition to a χ SDW insulator with a zero total Chern number but an anomalous ac Hall effect. The χ SDW is likely a generic phase of strongly correlated and highly frustrated hexagonal lattice electrons.
Higgins, David; Tweedale, Geoffrey
2010-01-01
In the Lancashire cotton textile industry, mule spinners were prone to a chronic and sometimes fatal skin cancer (often affecting the groin). The disease had reached epidemic proportions by the 1920s, which necessitated action by the government, employers, and trade unions. In contrast to previous accounts, this article focuses on the government's reaction to mule spinners' cancer. Using official records in the National Archives, the slow introduction of health and safety measures by the government is explored in detail. Although obstructionism by the employers played a key role, one of the reasons for government inaction was the ambiguity of scientific research on engineering oils. On the other hand, prolonged scientific research suited a government policy that was framed around self regulation - a policy that had proved largely ineffective by the 1950s. PMID:20734570
Aliouane, N.; Prokhnenko, O; Feyerherm, R; Mostovoy, M; Strempfer, J; Habicht, K; Rule, K; Dudzik, E; Wolter, A; et. al.
2008-01-01
Combining polarized and unpolarized neutron scattering techniques with x-ray resonant magnetic scattering we have studied the coupling between the Mn- and R-spin-ordering in the multiferroic RMnO3, R = Tb and Dy. Polarized neutron diffraction reveals the moment orientation associated with the various modes describing the complex magnetic ordering observed in TbMnO3, while neutron diffraction in high magnetic fields allows the identification of the origin (Mn versus Tb) of the various modes. In this way we identify significant Cx and Fz contributions from Tb arising from the coupling of Tb moments to the Mn cycloidal ordering. The x-ray studies give further insight into this coupling. In the ferroelectric phase, both TbMnO3 and DyMnO3 show an induced ordering of the R-ion with a propagation vector clamped to the Mn ordering. While in TbMnO3 this clamping leads to a ground state in which the two propagation vectors tTb and tMn obey the relation 3tTb-tMn = 1, in DyMnO3 the ferroelectric polarization is effectively enhanced. The theoretical analysis of these effects not only explains the observed behavior for R = Tb and Dy but can also be applied to understand the Mn-R interaction in the related compounds with R = Gd and Ho. Finally we show both experimentally and theoretically how the Mn-R coupling can enhance the ferroelectric polarization in this manganite's multiferroics.
Modulation of electronic properties from stacking orders and spin-orbit coupling for 3R-type MoS2.
Fan, Xiaofeng; Zheng, W T; Kuo, Jer-Lai; Singh, David J; Sun, C Q; Zhu, W
2016-01-01
Two-dimensional crystals stacked by van der Waals coupling, such as twisted graphene and coupled graphene-BN layers with unusual phenomena have been a focus of research recently. As a typical representative, with the modulation of structural symmetry, stacking orders and spin-orbit coupling, transitional metal dichalcogenides have shown a lot of fascinating properties. Here we reveal the effect of stacking orders with spin-orbit coupling on the electronic properties of few-layer 3R-type MoS2 by first principles methods. We analyze the splitting of states at the top of valence band and the bottom of conduction band, following the change of stacking order. We find that regardless of stacking orders and layers' number, the spin-up and spin-down channels are evidently separated and can be as a basis for the valley dependent spin polarization. With a model Hamiltonian about the layer's coupling, the band splitting can be effectively analyzed by the coupling parameters. It is found that the stacking sequences, such as abc and abca, have the stronger nearest-neighbor coupling which imply the popular of periodic abc stacking sequence in natural growth of MoS2. PMID:27053462
Modulation of electronic properties from stacking orders and spin-orbit coupling for 3R-type MoS2
Fan, Xiaofeng; Zheng, W. T.; Kuo, Jer-Lai; Singh, David J.; Sun, C.Q.; Zhu, W.
2016-01-01
Two-dimensional crystals stacked by van der Waals coupling, such as twisted graphene and coupled graphene-BN layers with unusual phenomena have been a focus of research recently. As a typical representative, with the modulation of structural symmetry, stacking orders and spin-orbit coupling, transitional metal dichalcogenides have shown a lot of fascinating properties. Here we reveal the effect of stacking orders with spin-orbit coupling on the electronic properties of few-layer 3R-type MoS2 by first principles methods. We analyze the splitting of states at the top of valence band and the bottom of conduction band, following the change of stacking order. We find that regardless of stacking orders and layers’ number, the spin-up and spin-down channels are evidently separated and can be as a basis for the valley dependent spin polarization. With a model Hamiltonian about the layer’s coupling, the band splitting can be effectively analyzed by the coupling parameters. It is found that the stacking sequences, such as abc and abca, have the stronger nearest-neighbor coupling which imply the popular of periodic abc stacking sequence in natural growth of MoS2. PMID:27053462
Modulation of electronic properties from stacking orders and spin-orbit coupling for 3R-type MoS2
NASA Astrophysics Data System (ADS)
Fan, Xiaofeng; Zheng, W. T.; Kuo, Jer-Lai; Singh, David J.; Sun, C. Q.; Zhu, W.
2016-04-01
Two-dimensional crystals stacked by van der Waals coupling, such as twisted graphene and coupled graphene-BN layers with unusual phenomena have been a focus of research recently. As a typical representative, with the modulation of structural symmetry, stacking orders and spin-orbit coupling, transitional metal dichalcogenides have shown a lot of fascinating properties. Here we reveal the effect of stacking orders with spin-orbit coupling on the electronic properties of few-layer 3R-type MoS2 by first principles methods. We analyze the splitting of states at the top of valence band and the bottom of conduction band, following the change of stacking order. We find that regardless of stacking orders and layers’ number, the spin-up and spin-down channels are evidently separated and can be as a basis for the valley dependent spin polarization. With a model Hamiltonian about the layer’s coupling, the band splitting can be effectively analyzed by the coupling parameters. It is found that the stacking sequences, such as abc and abca, have the stronger nearest-neighbor coupling which imply the popular of periodic abc stacking sequence in natural growth of MoS2.
Zhang, Q; Singh, K; Simon, C; Tung, L D; Balakrishnan, G; Hardy, V
2014-07-01
The orthovanadate DyVO_{3} crystal, known to exhibit multiple structural, spin-, and orbital-ordering transitions, is presently investigated on the basis of magnetization, heat capacity, resistivity, dielectric, and polarization measurements. Our main result is experimental evidence for the existence of multiferroicity below a high T_{C} of 108 K over a wide temperature range including different spin-orbital-ordered states. The onset of ferroelectricity is found to coincide with the antiferromagnetic C-type spin-ordering transition taking place at 108 K, which indicates that DyVO_{3} belongs to type-II multiferroics exhibiting a coupling between magnetism and ferroelectricity. Some anomalies detected on the temperature dependence of electric polarization are discussed with respect to the nature of the spin-orbital-ordered states of the V sublattice and the degree of spin alignment in the Dy sublattice. The orthovanadates RVO_{3} (R= rare earth or Y) form an important new category for searching for high-T_{C} multiferroics.
NASA Astrophysics Data System (ADS)
Ranjith, K. M.; Nath, R.; Majumder, M.; Kasinathan, D.; Skoulatos, M.; Keller, L.; Skourski, Y.; Baenitz, M.; Tsirlin, A. A.
2016-07-01
We report the thermodynamic properties, magnetic ground state, and microscopic magnetic model of the spin-1 frustrated antiferromagnet Li2NiW2O8 , showing successive transitions at TN 1≃18 K and TN 2≃12.5 K in zero field. Nuclear magnetic resonance and neutron diffraction reveal collinear and commensurate magnetic order with the propagation vector k =(1/2 ,0 ,1/2 ) below TN 2. The ordered moment of 1.8 μB at 1.5 K is directed along [0.89 (9 ),-0.10 (5 ),-0.49 (6 )] and matches the magnetic easy axis of spin-1 Ni2 + ions, which is determined by the scissor-like distortion of the NiO6 octahedra. Incommensurate magnetic order, presumably of spin-density-wave type, is observed in the region between TN 2 and TN 1. Density-functional band-structure calculations put forward a three-dimensional spin lattice with spin-1 chains running along the [01 1 ¯] direction and stacked on a spatially anisotropic triangular lattice in the a b plane. We show that the collinear magnetic order in Li2NiW2O8 is incompatible with the triangular lattice geometry and thus driven by a pronounced easy-axis single-ion anisotropy of Ni2 +.
NASA Astrophysics Data System (ADS)
Hague, J. P.; Chung, E. M. L.; Visser, D.; Balakrishnan, G.; Clementyev, E.; Paul, D. MK; Lees, M. R.
2005-11-01
We describe neutron inelastic scattering measurements of spin waves in the quasi-two-dimensional antiferromagnet FeTa2O6. The intrinsic spin wave dispersion for a single domain is deduced from linear spin wave theory and used to determine the intra-plane exchange coefficients. Almost dispersion-free excitations are observed along the c* direction perpendicular to the magnetic planes. This justifies the neglect of inter-plane coupling, which merely stabilizes the ordered configuration below TN. Spin wave theory yields values for the nearest neighbour and next nearest neighbour exchange constants on perpendicular diagonals of J = -0.040(9) meV, J'/J = 0.20(0), J''/J = 0.23(9), and the anisotropy parameter D = 0.31(8) meV. The large value of D shows an Ising-like spin configuration to be consistent with the experimental data. Measurements of the temperature dependence of the scattering show that magnetic excitations persist to at least 20 K (over two times TN) due to the extensive 2D short range order. This is a highly unusual result, and has consequences for the understanding of two-dimensional spin systems.
McGavin, Dennis G; Tennant, W Craighead
2009-06-17
In setting up a spin Hamiltonian (SH) to study high-spin Zeeman and high-spin nuclear and/or electronic interactions in electron paramagnetic resonance (EPR) experiments, it is argued that a maximally reduced SH (MRSH) framed in tesseral combinations of spherical tensor operators is necessary. Then, the SH contains only those terms that are necessary and sufficient to describe the particular spin system. The paper proceeds then to obtain interrelationships between the parameters of the MRSH and those of alternative SHs expressed in Cartesian tensor and Stevens operator-equivalent forms. The examples taken, initially, are those of Cartesian and Stevens' expressions for high-spin Zeeman terms of dimension BS(3) and BS(5). Starting from the well-known decomposition of the general Cartesian tensor of second rank to three irreducible tensors of ranks 0, 1 and 2, the decomposition of Cartesian tensors of ranks 4 and 6 are treated similarly. Next, following a generalization of the tesseral spherical tensor equations, the interrelationships amongst the parameters of the three kinds of expressions, as derived from equivalent SHs, are determined and detailed tables, including all redundancy equations, set out. In each of these cases the lowest symmetry, [Formula: see text] Laue class, is assumed and then examples of relationships for specific higher symmetries derived therefrom. The validity of a spin Hamiltonian containing mixtures of terms from the three expressions is considered in some detail for several specific symmetries, including again the lowest symmetry. Finally, we address the application of some of the relationships derived here to seldom-observed low-symmetry effects in EPR spectra, when high-spin electronic and nuclear interactions are present. PMID:21693947
2011-01-01
Purpose To theoretically develop and experimentally validate a formulism based on a fractional order calculus (FC) diffusion model to characterize anomalous diffusion in brain tissues measured with a twice-refocused spin-echo (TRSE) pulse sequence. Materials and Methods The FC diffusion model is the fractional order generalization of the Bloch-Torrey equation. Using this model, an analytical expression was derived to describe the diffusion-induced signal attenuation in a TRSE pulse sequence. To experimentally validate this expression, a set of diffusion-weighted (DW) images was acquired at 3 Tesla from healthy human brains using a TRSE sequence with twelve b-values ranging from 0 to 2,600 s/mm2. For comparison, DW images were also acquired using a Stejskal-Tanner diffusion gradient in a single-shot spin-echo echo planar sequence. For both datasets, a Levenberg-Marquardt fitting algorithm was used to extract three parameters: diffusion coefficient D, fractional order derivative in space β, and a spatial parameter μ (in units of μm). Using adjusted R-squared values and standard deviations, D, β and μ values and the goodness-of-fit in three specific regions of interest (ROI) in white matter, gray matter, and cerebrospinal fluid were evaluated for each of the two datasets. In addition, spatially resolved parametric maps were assessed qualitatively. Results The analytical expression for the TRSE sequence, derived from the FC diffusion model, accurately characterized the diffusion-induced signal loss in brain tissues at high b-values. In the selected ROIs, the goodness-of-fit and standard deviations for the TRSE dataset were comparable with the results obtained from the Stejskal-Tanner dataset, demonstrating the robustness of the FC model across multiple data acquisition strategies. Qualitatively, the D, β, and μ maps from the TRSE dataset exhibited fewer artifacts, reflecting the improved immunity to eddy currents. Conclusion The diffusion-induced signal
Critical spin fluctuations and the origin of nematic order in Ba(Fe1-xCox)2As2
NASA Astrophysics Data System (ADS)
Kretzschmar, F.; Böhm, T.; Karahasanović, U.; Muschler, B.; Baum, A.; Jost, D.; Schmalian, J.; Caprara, S.; Grilli, M.; di Castro, C.; Analytis, J. G.; Chu, J.-H.; Fisher, I. R.; Hackl, R.
2016-06-01
Nematic fluctuations and order play a prominent role in material classes such as the cuprates, some ruthenates or the iron-based compounds and may be interrelated with superconductivity. In iron-based compounds signatures of nematicity have been observed in a variety of experiments. However, the fundamental question as to the relevance of the related spin, charge or orbital fluctuations remains open. Here, we use inelastic light (Raman) scattering and study Ba(Fe1-xCox)2As2 (0 <= x <= 0.085) for getting direct access to nematicity and the underlying critical fluctuations with finite characteristic wavelengths. We show that the response from fluctuations appears only in B1g (x2 - y2) symmetry (1 Fe unit cell). The scattering amplitude increases towards the structural transition at Ts but vanishes only below the magnetic ordering transition at TSDW < Ts, suggesting a magnetic origin of the fluctuations. The theoretical analysis explains the selection rules and the temperature dependence of the fluctuation response. These results make magnetism the favourite candidate for driving the series of transitions.
NASA Astrophysics Data System (ADS)
De, Santanu; Kumar, Kranti; Banerjee, A.; Chaddah, P.
2016-05-01
We have found that the geometrically frustrated spin chain compound Ca3Co2O6 belonging to Ising like universality class with uniaxial anisotropy shows kinetic arrest of first order intermediate phase (IP) to ferrimagnetic (FIM) transition. In this system, dc magnetization measurements followed by different protocols suggest the coexistence of high temperature IP with equilibrium FIM phase in low temperature. Formation of metastable state due to hindered first order transition has also been probed through cooling and heating in unequal field (CHUF) protocol. Kinetically arrested high temperature IP appears to persist down to almost the spin freezing temperature in this system.
NASA Astrophysics Data System (ADS)
Kumar, Manoranjan; Soos, Z. G.
2013-10-01
The quantum phases of one-dimensional spin s=1/2 chains are discussed for models with two parameters, frustrating exchange g=J2>0 between second neighbors and normalized nonfrustrating power-law exchange with exponent α and distance dependence r-α. The ground state (GS) at g=0 has a long-range order (LRO) for α<2 and long-range spin fluctuations for α>2. The models conserve total spin S=SA+SB, have singlet GS for any g, α≥0 and decouple at 1/g=0 to linear Heisenberg antiferromagnets on sublattices A and B of odd- and even-numbered sites. Exact diagonalization of finite chains gives the sublattice spin
Zhang, Qiang; Fernandes, Rafael M.; Lamsal, Jagat; Yan, Jiaqiang; Chi, Songxue; Tucker, Gregory S.; Pratt, Daniel K.; Lynn, Jeffrey W.; McCallum, R. W.; Canfield, Paul C.; Lograsso, Thomas A.; Goldman, Alan I.; Vaknin, David; McQueeney, Robert J.
2015-02-04
Inelastic neutron scattering is employed to investigate the impact of electronic nematic order on the magnetic spectra of LaFeAsO and Ba(Fe_{0.953}Co_{0.047})_{2}As_{2}. These materials are ideal to study the paramagnetic-nematic state, since the nematic order, signaled by the tetragonal-to-orthorhombic transition at T_{S}, sets in well above the stripe antiferromagnetic ordering at T_{N}. We find that the temperature-dependent dynamic susceptibility displays an anomaly at T_{S} followed by a sharp enhancement in the spin-spin correlation length, revealing a strong feedback effect of nematic order on the low-energy magnetic spectrum. As a result, our findings can be consistently described by a model that attributes the structural or nematic transition to magnetic fluctuations, and unveils the key role played by nematic order in promoting the long-range stripe antiferromagnetic order in iron pnictides.
Unstable spin-ice order in the stuffed metallic pyrochlore Pr2+xIr2-xO7-δ
MacLaughlin, D. E.; Bernal, O. O.; Shu, Lei; Ishikawa, Jun; Matsumoto, Yosuke; Wen, Jia -Jia; Mourigal, Martin P.; Stock, C.; Ehlers, Georg; Broholm, C. L.; et al
2015-08-24
Specific heat, elastic neutron scattering, and muon spin rotation experiments have been carried out on a well-characterized sample of “stuffed” (Pr-rich) Pr2+xIr2-xO7-δ. Elastic neutron scattering shows the onset of long-range spin-ice “2-in/2-out” magnetic order at 0.93 kelvin, with an ordered moment of 1.7(1) Bohr magnetons per Pr ion at low temperatures. Approximate lower bounds on the correlation length and correlation time in the ordered state are 170 angstroms and 0.7 nanosecond, respectively. Muon spin rotation experiments yield an upper bound 2.6(7) milliteslas on the local field B4floc at the muon site, which is nearly two orders of magnitude smaller thanmore » the expected dipolar field for long-range spin-ice ordering of 1.7-Bohr magneton moments (120–270 milliteslas, depending on the muon site). This shortfall is due in part to splitting of the non-Kramers crystal-field ground-state doublets of near-neighbor Pr3+ ions by the positive-muon-induced lattice distortion. For this to be the only effect, however, ~160 Pr moments out to a distance of ~14 angstroms must be suppressed. An alternative scenario—one consistent with the observed reduced nuclear hyperfine Schottky anomaly in the specific heat—invokes slow correlated Pr-moment fluctuations in the ordered state that average B4floc on the μSR time scale (~10-7 second), but are static on the time scale of the elastic neutron scattering experiments (~10-9 second). In this picture, the dynamic muon relaxation suggests a Pr3+ 4f correlation time of a few nanoseconds, which should be observable in a neutron spin echo experiment.« less
Lochan, Rohini C.; Head-Gordon, Martin
2007-01-01
Coupled cluster methods based on Brueckner orbitals are well-known to resolve the problems of symmetry-breaking and spin-contamination that are often associated with Hartree-Fock orbitals. However their computational cost is large enough to prevent application to large molecules. Here they present a simple approximation where the orbitals are optimized with the mean-field energy plus a correlation energy taken as the opposite-spin component of the second order many-body correlation energy, scaled by an empirically chosen parameter (recommended as 1.2 for general applications). This optimized 2nd order opposite spin (abbreviated as O2) method requires fourth order computation on each orbital iteration. O2 is shown to yield predictions of structure and frequencies for closed shell molecules that are very similar to scaled second order Moller-Plesset methods. However it yields substantial improvements for open shell molecules, where problems with spin-contamination and symmetry breaking are shown to be greatly reduced.
NASA Astrophysics Data System (ADS)
Oravova, Lucie; Zhang, Zhiying; Church, Nathan; Harrison, Richard J.; Howard, Christopher J.; Carpenter, Michael A.
2013-03-01
Hematite, Fe2O3, provides in principle a model system for multiferroic (ferromagnetic/ferroelastic) behavior at low levels of strain coupling. The elastic and anelastic behavior associated with magnetic phase transitions in a natural polycrystalline sample have therefore been studied by resonant ultrasound spectroscopy (RUS) in the temperature range from 11 to 1072 K. Small changes in softening and attenuation are interpreted in terms of weak but significant coupling of symmetry-breaking and non-symmetry-breaking strains with magnetic order parameters in the structural sequence R\\overline{3}c{1}^{\\prime}\\rightarrow C 2/c\\rightarrow R\\overline{3}c. The R\\overline{3}c{1}^{\\prime}\\rightarrow C 2/c transition at TN = 946 ± 1 K is an example of a multiferroic transition which has both ferromagnetic (from canting of antiferromagnetically ordered spin moments) and ferroelastic (rhombohedral → monoclinic) character. By analogy with the improper ferroelastic transition in Pb3(PO4)2, W and W‧ ferroelastic twin walls which are also 60° and 120° magnetic domain walls should develop. These have been tentatively identified from microstructures reported in the literature. The very low attenuation in the stability field of the C2/c structure in the polycrystalline sample used in the present study, in comparison with the strong acoustic dissipation reported for single crystal samples, implies, however, that the individual grains each consist of a single ferroelastic domain or that the twin walls are strongly pinned by grain boundaries. This absence of attenuation allows an intrinsic loss mechanism associated with the transition point to be seen and interpreted in terms of local coupling of shear strains with fluctuations which have relaxation times in the vicinity of ˜10-8 s. The first order C 2/c\\rightarrow R\\overline{3}c (Morin) transition occurs through a temperature interval of coexisting phases but the absence of an acoustic loss peak suggests that the
Chi, Songxue; Ye, F.; Dai, Pengcheng; Fernandez-Baca, J. A.; Huang, Q.; Lynn, J. W.; Plummer, E. W.; Mathieu, R.; Kaneko, Y.; Tokura, Y.
2007-01-01
We use neutron scattering to study the lattice and magnetic structure of the layered half-doped manganite Pr0.5Ca1.5MnO4. On cooling from high temperature, the system first becomes charge-and orbital-ordered (CO/OO) near TCO = 300 K and then develops checkerboard-like antiferromagnetic (AF) order below TN = 130 K. At temperatures above TN but below TCO (TN
Chi, Songxue; Ye, Feng; Dai, Pengcheng; Fernandez-Baca, Jaime A; Huang, Q.; Lynn, J. W.; Plummer, E Ward; Mathieu, R.; Kaneko, Y.; Tokura, Y.
2007-01-01
We use neutron scattering to study the lattice and magnetic structure of the layered half-doped manganite Pr0.5Ca1.5MnO4. On cooling from high temperature, the system first becomes chargeand orbital-ordered (CO/OO) near TCO = 300 K and then develops checkerboard-like antiferromagnetic (AF) order below TN = 130 K. At temperatures above TN but below TCO (TN
Collinear order in the frustrated three-dimensional spin-1/2 antiferromagnet Li2CuW2O8
NASA Astrophysics Data System (ADS)
Ranjith, K. M.; Nath, R.; Skoulatos, M.; Keller, L.; Kasinathan, D.; Skourski, Y.; Tsirlin, A. A.
2015-09-01
Magnetic frustration in three dimensions (3D) manifests itself in the spin-1/2 insulator Li2CuW2O8 . Density-functional band-structure calculations reveal a peculiar spin lattice built of triangular planes with frustrated interplane couplings. The saturation field of 29 T contrasts with the susceptibility maximum at 8.5 K and a relatively low Néel temperature TN≃3.9 K . Magnetic order below TN is collinear with the propagation vector (0 ,1/2 ,0 ) and an ordered moment of 0.65(4) μB according to neutron diffraction data. This reduced ordered moment together with the low maximum of the magnetic specific heat (Cmax/R ≃0.35 ) pinpoint strong magnetic frustration in 3D. Collinear magnetic order suggests that quantum fluctuations play a crucial role in this system, where a noncollinear spiral state would be stabilized classically.
Code of Federal Regulations, 2010 CFR
2010-01-01
... military service members and veterans; (iii) marketing the Federal Government as an employer of choice to transitioning service members and veterans; (iv) marketing the talent, experience, and dedication...
Bordbar, G. H.; Rezaei, Z.; Montakhab, Afshin
2011-04-15
In this article, the lowest order constrained variational method is used to investigate the magnetic properties of spin-polarized neutron matter in the presence of strong magnetic field at zero temperature employing the AV{sub 18} potential. Our results indicate that a ferromagnetic phase transition is induced by a strong magnetic field with strength greater than 10{sup 18} G, leading to a partial spin polarization of the neutron matter. It is also shown that the equation of state of neutron matter in the presence of a magnetic field is stiffer than in the absence of a magnetic field.
NASA Astrophysics Data System (ADS)
Willenberg, B.; Schäpers, M.; Wolter, A. U. B.; Drechsler, S.-L.; Reehuis, M.; Hoffmann, J.-U.; Büchner, B.; Studer, A. J.; Rule, K. C.; Ouladdiaf, B.; Süllow, S.; Nishimoto, S.
2016-01-01
Low-temperature neutron diffraction and NMR studies of field-induced phases in linarite are presented for magnetic fields H ∥b axis. A two-step spin-flop transition is observed, as well as a transition transforming a helical magnetic ground state into an unusual magnetic phase with sine-wave-modulated moments ∥H . An effective J˜ 1-J˜ 2 single-chain model with a magnetization-dependent frustration ratio αeff=-J˜2/J˜1 is proposed. The latter is governed by skew interchain couplings and shifted to the vicinity of the ferromagnetic critical point. It explains qualitatively the observation of a rich variety of exotic longitudinal collinear spin-density wave, SDWp , states (9 ≥p ≥2 ).
Tanamoto, Tetsufumi; Ono, Keiji; Liu, Yu-xi; Nori, Franco
2015-01-01
Hamiltonian engineering is an important approach for quantum information processing, when appropriate materials do not exist in nature or are unstable. So far there is no stable material for the Kitaev spin Hamiltonian with anisotropic interactions on a honeycomb lattice, which plays a crucial role in the realization of both Abelian and non-Abelian anyons. Here, we show two methods to dynamically realize the Kitaev spin Hamiltonian from the conventional Heisenberg spin Hamiltonian using pulse-control techniques based on the Baker-Campbell-Hausdorff (BCH) formula. In the first method, the Heisenberg interaction is changed into Ising interactions in the first process of the pulse sequence. In the next process of the first method, we transform them to a desirable anisotropic Kitaev spin Hamiltonian. In the second more efficient method, we show that if we carefully design two-dimensional pulses that vary depending on the qubit location, we can obtain the desired Hamiltonian in only one step of applying the BCH formula. As an example, we apply our methods to spin qubits based on quantum dots, in which the effects of both the spin-orbit interaction and the hyperfine interaction are estimated. PMID:26081899
Rybkin, Vladimir V; VandeVondele, Joost
2016-05-10
To obtain consistent geometries for the computation of properties, nuclear gradients are essential. Here, we report a fully periodic Γ-point, massively parallel implementation of spin-unrestricted second-order Møller-Plesset (MP2) forces. It is based on the resolution-of-identity and Gaussian and plane waves approach to calculate electron repulsion integrals and is made available in the CP2K program. The algorithm is optimized for modern supercomputer architectures and is capable of employing both CPUs and GPUs. The asymptotic computational scaling is O(N(5)), which is observed for the systems containing more than 100 second-row atoms with triple-ζ quality basis sets. For smaller systems, the energy and forces can be evaluated within minutes; for bigger systems within hours, provided that thousands of processor units are available. Spin-unrestricted MP2 calculations are, computationally, ∼3 times more demanding than spin-restricted ones, but exhibit a better parallel performance. As a bonus, the gradient implementation allows for computing spin-density distributions not available in energy calculations. The method has been successfully used for computing the crystal structure of the TEMPO radical and to obtain the spin density distribution of an F-center in lithium fluoride at a consistent geometry. We expect this computationally efficient tool to be useful for the chemistry, materials science, and solid-state physics communities. PMID:27018709
Strečka, Jozef; Ekiz, Cesur
2015-05-01
The geometrically frustrated spin-1/2 Ising-Heisenberg model on triangulated Husimi lattices is exactly solved by combining the generalized star-triangle transformation with the method of exact recursion relations. The ground-state and finite-temperature phase diagrams are rigorously calculated along with both sublattice magnetizations of the Ising and Heisenberg spins. It is evidenced that the Ising-Heisenberg model on triangulated Husimi lattices with two or three interconnected triangles-in-triangles units displays in a highly frustrated region a quantum disorder irrespective of temperature, whereas the same model on triangulated Husimi lattices with a greater connectivity of triangles-in-triangles units exhibits at low enough temperatures an outstanding quantum order due to the order-by-disorder mechanism. The quantum reduction of both sublattice magnetizations in the peculiar quantum ordered state gradually diminishes upon increasing the coordination number of the underlying Husimi lattice. PMID:26066155
Unstable spin-ice order in the stuffed metallic pyrochlore Pr2 +xIr2 -xO7 -δ
NASA Astrophysics Data System (ADS)
MacLaughlin, D. E.; Bernal, O. O.; Shu, Lei; Ishikawa, Jun; Matsumoto, Yosuke; Wen, J.-J.; Mourigal, M.; Stock, C.; Ehlers, G.; Broholm, C. L.; Machida, Yo; Kimura, Kenta; Nakatsuji, Satoru; Shimura, Yasuyuki; Sakakibara, Toshiro
2015-08-01
Specific heat, elastic neutron scattering, and muon spin rotation (μ SR ) experiments have been carried out on a well-characterized sample of "stuffed" (Pr-rich) Pr2 +xIr2 -xO7 -δ . Elastic neutron scattering shows the onset of long-range spin-ice "2-in/2-out" magnetic order at TM=0.93 K, with an ordered moment of 1.7 (1 )μB/ Pr ion at low temperatures. Approximate lower bounds on the correlation length and correlation time in the ordered state are 170 Å and 0.7 ns, respectively. μ SR experiments yield an upper bound 2.6(7) mT on the local field Bloc4 f at the muon site, which is nearly two orders of magnitude smaller than the expected dipolar field for long-range spin-ice ordering of 1.7 μB moments (120-270 mT, depending on muon site). This shortfall is due in part to splitting of the non-Kramers crystal-field ground-state doublets of near-neighbor Pr3 + ions by the μ+-induced lattice distortion. For this to be the only effect, however, ˜160 Pr moments out to a distance of ˜14 Å must be suppressed. An alternative scenario, which is consistent with the observed reduced nuclear hyperfine Schottky anomaly in the specific heat, invokes slow correlated Pr-moment fluctuations in the ordered state that average Bloc4 f on the μ SR time scale (˜10-7s) , but are static on the time scale of the elastic neutron scattering experiments (˜10-9s) . In this picture, the dynamic muon relaxation suggests a Pr3 +4 f correlation time of a few nanoseconds, which should be observable in a neutron spin echo experiment.
Spin noise spectroscopy in semiconductors: from a billion down to single spins
NASA Astrophysics Data System (ADS)
Hübner, J.; Dahbashi, R.; Berski, F.; Wiegand, J.; Kuhn, H.; Lonnemann, J.; Oestreich, M.
2014-08-01
Spin noise spectroscopy in semiconductors has matured during the past nine years into a versatile and well developed technique being capable to unveil the intrinsic and unaltered spin dynamics in a wide range of semiconductor systems. Originating from atom and quantum optics as a potential true quantum non-demolition measurement technique, SNS is capable of unearthing the intricate dynamics of free or localized electron and hole spins in semiconductors being eventually coupled to the nuclear spin bath as well. In this contribution, we review shortly the major steps which inspired the success of spin noise spectroscopy in semiconductors and present the most recent extensions into the low-invasive detection regime of the spin dynamics for the two extreme limits of very high and extremely low rates of spin decoherence, respectively. On the one hand, merging ultrafast laser spectroscopy with spin noise spectroscopy enables the detection of spin noise with picosecond resolution, i.e., with THz bandwidths yielding access to otherwise concealed microscopic electronic processes. On the other hand, we present very high sensitivity SNS being capable to measure the extremely long spin coherence of single holes enclosed in individual quantum dots venturing a step forward towards true optical quantum non-demolition experiments in semiconductors. In addition, higher-order spin noise statistics of, e.g., single charges can give information beyond the linear response regime governed by the fundamental fluctuationdissipation theorem and thereby possibly shed some light on the nested coupling between electronic and nuclear spins.
Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4
Jacobsen, H.; Zaliznyak, I. A.; Savici, A. T.; Winn, B. L.; Chang, S.; Hücker, M.; Gu, G. D.; Tranquada, J. M.
2015-11-20
Tmore » he relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La1.93Sr0.07CuO4 a superconductor with a transition temperature of c = 20 K. At << c, we find incommensurate spin fluctuations with a quasielastic energy spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below ~ 10 K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO6 octahedra about Cu-O bonds, which are associated with inequivalent O sites within the CuO2 planes. Moreover, we observed a weak elastic (3 ⁻30) superlattice peak that implies a reduced lattice symmetry. he presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped La2-xSrxCuO4. he coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.« less
Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4
Jacobsen, H; Zaliznyak, Igor; Savici, Andrei T; Winn, Barry L; Chang, S; Hucker, M.; Gu, Genda; Tranquada, John M.
2015-01-01
The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La1.93Sr0.07CuO4, a superconductor with a transition temperature of Tc=20 K. At T Tc, we find incommensurate spin fluctuations with a nearly energy-independent spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below 10 K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO6 octahedra about Cu-O bonds, which are associated with inequivalent O sites within the CuO2 planes. Furthermore, we observed a weak elastic (33 0) superlattice peak that implies a reduced lattice symmetry. The presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped La2 xSrxCuO4. The coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.
Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4
Jacobsen, H; Zaliznyak, Igor; Savici, Andrei T; Winn, Barry L; Chang, S; Hucker, M.; Gu, Genda; Tranquada, John M.
2015-01-01
The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La1.93Sr0.07CuO4, a superconductor with a transition temperature of Tc=20 K. At T Tc, we find incommensurate spin fluctuations with a nearly energy-independent spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below 10 K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO6 octahedra about Cu-O bonds, which are associated with inequivalent Omore » sites within the CuO2 planes. Furthermore, we observed a weak elastic (33 0) superlattice peak that implies a reduced lattice symmetry. The presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped La2 xSrxCuO4. The coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.« less
NASA Astrophysics Data System (ADS)
Ghorbani, Elaheh; Tocchio, Luca F.; Becca, Federico
2016-02-01
By using variational wave functions and quantum Monte Carlo techniques, we investigate the complete phase diagram of the Heisenberg model on the anisotropic triangular lattice, where two out of three bonds have superexchange couplings J and the third one has instead J'. This model interpolates between the square lattice and the isotropic triangular one, for J'/J ≤1 , and between the isotropic triangular lattice and a set of decoupled chains, for J /J'≤1 . We consider all the fully symmetric spin liquids that can be constructed with the fermionic projective-symmetry group classification (Zhou and Wen, arXiv:cond-mat/0210662) and we compare them with the spiral magnetic orders that can be accommodated on finite clusters. Our results show that, for J'/J ≤1 , the phase diagram is dominated by magnetic orderings, even though a spin-liquid state may be possible in a small parameter window, i.e., 0.7 ≲J'/J ≲0.8 . In contrast, for J /J'≤1 , a large spin-liquid region appears close to the limit of decoupled chains, i.e., for J /J'≲0.6 , while magnetically ordered phases with spiral order are stabilized close to the isotropic point.
NASA Astrophysics Data System (ADS)
Edén, Mattias
2002-12-01
Order-selective multiple-quantum excitation in magic-angle spinning nuclear magnetic resonance is explored using a class of symmetry-based pulse sequences, denoted S Mχ. Simple rules are presented that aid the design of S Mχ schemes with certain desirable effective Hamiltonians. They are applied to construct sequences generating trilinear effective dipolar Hamiltonians, suitable for efficient excitation of triple-quantum coherences in rotating solids. The new sequences are investigated numerically and demonstrated by 1H experiments on adamantane.
Disorder from order among anisotropic next-nearest-neighbor Ising spin chains in SrHo_{2}O_{4}
Wen, J. -J.; Tian, W.; Garlea, V. O.; Koohpayeh, S. M.; McQueen, T. M.; Li, H. -F.; Yan, J. -Q.; Rodriguez-Rivera, J. A.; Vaknin, D.; Broholm, C. L.
2015-02-26
In this study, we describe why Ising spin chains with competing interactions in SrHo_{2}O_{4} segregate into ordered and disordered ensembles at low temperatures (T). Using elastic neutron scattering, magnetization, and specific heat measurements, the two distinct spin chains are inferred to have Néel (↑↓↑↓) and double-Néel (↑↑↓↓) ground states, respectively. Below T_{N} = 0.68(2)K, the Néel chains develop three-dimensional long range order (LRO), which arrests further thermal equilibration of the double-Néel chains so they remain in a disordered incommensurate state for T below T_{S} = 0.52(2)K. SrHo_{2}O_{4} distills an important feature of incommensurate low dimensional magnetism: kinetically trapped topological defects in a quasi–d–dimensional spin system can preclude order in d + 1 dimensions.
Moudden, A.H.; Hennion, B. - Centre d'Etudes Nucleaires de Saclay, 91 - Gif-sur-Yvette ); Schweiss, P. - Centre d'Etudes Nucleaires de Saclay, 91 - Gif-sur-Yvette Kernforschungszentrum Karlsruhe GmbH . Inst. fuer Nukleare Festkoerperphysik); Gehring, P.M.; Shirane, G. (Brookhaven National Lab., Upton, NY (
1991-01-01
Elastic neutron scattering experiments performed on single crystals of Nd{sub 1.5}Ba{sub 1.5}Cu{sub 3}O{sub 6+y} reveal successive antiferromagnetic (AF) ordering of the Cu{sup ++} spins. The as grown single crystals show an AF structure characterized by a Neel temperature T{sub N1} {approximately} 390K and a magnetic wave vector (1/2 1/2 0) referring to the tetragonal structure of NdBa{sub 2}Cu{sub 3}O{sub 6}. As the temperature is lowered below T{sub N2} {approximately} 150K, a spin reorientation develops and a second AF ordering with (1/2 1/2 1/2) wave vector is stabilized. When the samples are oxygenated the tetragonal symmetry and the Neel temperature T{sub N1} remain unchanged, whereas the spin reorientation at T{sub N2} is suppressed. The results indicate that the Nd/Ba substitution increases the stability of the tetragonal structure upon the oxygen content. This may induce new possibilities of local oxygen ordering that favour the presence of holes in the deficient layer.
Strong enhancement of spin ordering by A -site magnetic ions in the ferrimagnet CaC u3F e2O s2O12
NASA Astrophysics Data System (ADS)
Deng, Hongshan; Liu, Min; Dai, Jianhong; Hu, Zhiwei; Kuo, Changyang; Yin, Yunyu; Yang, Junye; Wang, Xiao; Zhao, Qing; Xu, Yuanji; Fu, Zhaoming; Cai, Jianwang; Guo, Haizhong; Jin, Kuijuan; Pi, Tunwen; Soo, Yunliang; Zhou, Guanghui; Cheng, Jinguang; Chen, Kai; Ohresser, Philippe; Yang, Yi-feng; Jin, Changqing; Tjeng, Liu-Hao; Long, Youwen
2016-07-01
A B O3 perovskite is a kind of very important functional material with versatile physical properties. Although B -site chemical substitution with various magnetic ions has been widely investigated, the A -site doping with magnetic transition metal is little known. Here we report A A3'B2B2'O12 -type A - and B -site ordered ferrimagnet CaC u3F e2O s2O12 with magnetic transition metals occupying three different atomic sites (A', B , and B' sites). This compound is synthesized by a special high-pressure annealing process. It possesses a much higher Curie temperature TC of 580 K compared with that of the B -site-only ordered C a2FeOs O6 (TC=320 K ) without magnetic ion at the A site. First-principles numerical calculations reveal that this enhancement primarily originates from the additional spin interaction between the A'-site C u2 + and the B'-site O s5 + , generating a strong C u2 +(↑) F e3 +(↑) O s5 +(↓) ferrimagnetic spin coupling. This work opens up an alternative way for enhancing the spin ordering temperature by introducing A -site magnetic ions.
Prosdocimi, Francisco; Bittencourt, Daniela; da Silva, Felipe Rodrigues; Kirst, Matias; Motta, Paulo C.; Rech, Elibio L.
2011-01-01
Characterized by distinctive evolutionary adaptations, spiders provide a comprehensive system for evolutionary and developmental studies of anatomical organs, including silk and venom production. Here we performed cDNA sequencing using massively parallel sequencers (454 GS-FLX Titanium) to generate ∼80,000 reads from the spinning gland of Actinopus spp. (infraorder: Mygalomorphae) and Gasteracantha cancriformis (infraorder: Araneomorphae, Orbiculariae clade). Actinopus spp. retains primitive characteristics on web usage and presents a single undifferentiated spinning gland while the orbiculariae spiders have seven differentiated spinning glands and complex patterns of web usage. MIRA, Celera Assembler and CAP3 software were used to cluster NGS reads for each spider. CAP3 unigenes passed through a pipeline for automatic annotation, classification by biological function, and comparative transcriptomics. Genes related to spider silks were manually curated and analyzed. Although a single spidroin gene family was found in Actinopus spp., a vast repertoire of specialized spider silk proteins was encountered in orbiculariae. Astacin-like metalloproteases (meprin subfamily) were shown to be some of the most sampled unigenes and duplicated gene families in G. cancriformis since its evolutionary split from mygalomorphs. Our results confirm that the evolution of the molecular repertoire of silk proteins was accompanied by the (i) anatomical differentiation of spinning glands and (ii) behavioral complexification in the web usage. Finally, a phylogenetic tree was constructed to cluster most of the known spidroins in gene clades. This is the first large-scale, multi-organism transcriptome for spider spinning glands and a first step into a broad understanding of spider web systems biology and evolution. PMID:21738742
NASA Astrophysics Data System (ADS)
Hrovat, Matevž Majcen; Jeglič, Peter; Klanjšek, Martin; Hatakeda, Takehiro; Noji, Takashi; Tanabe, Yoichi; Urata, Takahiro; Huynh, Khuong K.; Koike, Yoji; Tanigaki, Katsumi; Arčon, Denis
2015-09-01
The superconducting critical temperature, Tc, of FeSe can be dramatically enhanced by intercalation of a molecular spacer layer. Here we report on a 77Se,7Li , and 1H nuclear magnetic resonance (NMR) study of the powdered hyper-interlayer-expanded Lix(C2H8N2) yFe2 -zSe2 with a nearly optimal Tc=45 K. The absence of any shift in the 7Li and 1H NMR spectra indicates a complete decoupling of interlayer units from the conduction electrons in FeSe layers, whereas nearly temperature-independent 7Li and 1H spin-lattice relaxation rates are consistent with the non-negligible concentration of Fe impurities present in the insulating interlayer space. On the other hand, the strong temperature dependence of 77Se NMR shift and spin-lattice relaxation rate, 1 /77T1 , is attributed to the holelike bands close to the Fermi energy. 1 /77T1 shows no additional anisotropy that would account for the onset of electronic nematic order down to Tc. Similarly, no enhancement in 1 /77T1 due to the spin fluctuations could be found in the normal state. Yet, a characteristic power-law dependence 1 /77T1∝T4.5 still complies with the Cooper pairing mediated by spin fluctuations.
Wang, C; Stojić, N; Binggeli, N
2014-10-01
The spin-ordering and electronic properties of the c(2 × 2) MnCu/Cu(1 1 0) surface alloy are investigated by means of ab initio density-functional calculations. We first address the magnetic ground state and the robustness of the spin-polarization properties. The lowest-energy state is found to be ferromagnetic with a very low Curie temperature, showing that the paramagnetic phase should be established in this system at room temperature. The calculated trends obtained for the various spin structures considered indicate that the local Mn-spin moment and resulting reduced work function as well as Mn-outward buckling should persist in the paramagnetic phase. We then address the electronic surface-band structure of the paramagnetic phase close to the Fermi energy, in connection with the interpretation of recent angle-resolved-photoemission-spectroscopy experiments at room temperature. Our calculations account for an intriguing new surface-band feature observed experimentally near the [Formula: see text] point upon alloy formation, and provide a microscopic interpretation for this feature and for the alloy-induced changes in the Cu(1 1 0) Shockley surface state. PMID:25158692
Federal Register 2010, 2011, 2012, 2013, 2014
2011-05-17
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2012-01-01
... 745 and rules on animal acquisition, transport, care, handling and use in 9 CFR parts 1 through 4... Government-wide common rule that the DOE has codified at 10 CFR part 601. The “List of Certifications and... Act of 1964 (42 U.S.C. 2000d, et seq.) as implemented by DOE regulations at 10 CFR part 1040....
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2013-01-01
... 745 and rules on animal acquisition, transport, care, handling and use in 9 CFR parts 1 through 4... Government-wide common rule that the DOE has codified at 10 CFR part 601. The “List of Certifications and... Act of 1964 (42 U.S.C. 2000d, et seq.) as implemented by DOE regulations at 10 CFR part 1040....
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2013-01-01
... Extracted From Nuclear Weapons 13617 Order 13617 Presidential Documents Executive Orders Executive Order... to the Disposition of Highly Enriched Uranium Extracted From Nuclear Weapons By the authority vested... accumulation of a large volume of weapons-usable fissile material in the territory of the Russian...
Moderate positive spin Hall angle in uranium
NASA Astrophysics Data System (ADS)
Singh, Simranjeet; Anguera, Marta; del Barco, Enrique; Springell, Ross; Miller, Casey W.
2015-12-01
We report measurements of spin pumping and the inverse spin Hall effect in Ni80Fe20/uranium bilayers designed to study the efficiency of spin-charge interconversion in a super-heavy element. We employ broad-band ferromagnetic resonance on extended films to inject a spin current from the Ni80Fe20 (permalloy) into the uranium layer, which is then converted into an electric field by the inverse spin Hall effect. Surprisingly, our results suggest a spin mixing conductance of order 2 × 1019 m-2 and a positive spin Hall angle of 0.004, which are both merely comparable with those of several transition metals. These results thus support the idea that the electronic configuration may be at least as important as the atomic number in governing spin pumping across interfaces and subsequent spin Hall effects. In fact, given that both the magnitude and the sign are unexpected based on trends in d-electron systems, materials with unfilled f-electron orbitals may hold additional exploration avenues for spin physics.
Moderate positive spin Hall angle in uranium
Singh, Simranjeet; Anguera, Marta; Barco, Enrique del E-mail: cwmsch@rit.edu; Springell, Ross; Miller, Casey W. E-mail: cwmsch@rit.edu
2015-12-07
We report measurements of spin pumping and the inverse spin Hall effect in Ni{sub 80}Fe{sub 20}/uranium bilayers designed to study the efficiency of spin-charge interconversion in a super-heavy element. We employ broad-band ferromagnetic resonance on extended films to inject a spin current from the Ni{sub 80}Fe{sub 20} (permalloy) into the uranium layer, which is then converted into an electric field by the inverse spin Hall effect. Surprisingly, our results suggest a spin mixing conductance of order 2 × 10{sup 19} m{sup −2} and a positive spin Hall angle of 0.004, which are both merely comparable with those of several transition metals. These results thus support the idea that the electronic configuration may be at least as important as the atomic number in governing spin pumping across interfaces and subsequent spin Hall effects. In fact, given that both the magnitude and the sign are unexpected based on trends in d-electron systems, materials with unfilled f-electron orbitals may hold additional exploration avenues for spin physics.
Disappearance of static magnetic order and evolution of spin fluctuations in Fe_{1+δ}Se_{x}Te_{1-x}
Xu, Zhijun; Wen, Jinsheng; Xu, Guangyong; Jie, Qing; Lin, Zhiwei; Li, Qiang; Chi, Songxue; Singh, D. K.; Gu, Genda; Tranquada, John M.
2010-09-29
We report neutron-scattering studies on static magnetic orders and spin excitations in the Fe-based chalcogenide system Fev Se_{1+δ} Te_{1-x} with different Fe and Se compositions. Short-range static magnetic order with an in-plane wave vector near the (0.5,0) (using the two-Fe unit cell), together with strong low-energy magnetic excitations is found in all nonsuperconducting samples for Se doping up to 45%. When the static order disappears and bulk superconductivity emerges, the spectral weight of the magnetic excitations shifts to the region of reciprocal space near the in-plane wave vector (0.5, 0.5), corresponding to “collinear” spin correlations. Our results suggest that there is a strong correlation between superconductivity and the character of the magnetic order/fluctuations in this system. Excess Fe appears to be important for stabilizing the magnetic order that competes with superconductivity.
Code of Federal Regulations, 2011 CFR
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Code of Federal Regulations, 2010 CFR
2010-01-01
... Government-wide common rule that the DOE has codified at 10 CFR part 601. The “List of Certifications and... Act of 1964 (42 U.S.C. 2000d, et seq.) as implemented by DOE regulations at 10 CFR part 1040. These... Discrimination Act of 1975 (42 U.S.C. 6101, et seq.) as implemented by DOE regulations at 10 CFR part 1040....
Datta, Dipayan Gauss, Jürgen
2014-09-14
An analytic scheme is presented for the evaluation of first derivatives of the energy for a unitary group based spin-adapted coupled cluster (CC) theory, namely, the combinatoric open-shell CC (COSCC) approach within the singles and doubles approximation. The widely used Lagrange multiplier approach is employed for the derivation of an analytical expression for the first derivative of the energy, which in combination with the well-established density-matrix formulation, is used for the computation of first-order electrical properties. Derivations of the spin-adapted lambda equations for determining the Lagrange multipliers and the expressions for the spin-free effective density matrices for the COSCC approach are presented. Orbital-relaxation effects due to the electric-field perturbation are treated via the Z-vector technique. We present calculations of the dipole moments for a number of doublet radicals in their ground states using restricted open-shell Hartree-Fock (ROHF) and quasi-restricted HF (QRHF) orbitals in order to demonstrate the applicability of our analytic scheme for computing energy derivatives. We also report calculations of the chlorine electric-field gradients and nuclear quadrupole-coupling constants for the CCl, CH{sub 2}Cl, ClO{sub 2}, and SiCl radicals.
Ewings, Russell A.; Perring, T. G.; Sikora, O.; Abernathy, Douglas L; Tomioka, Y.; Tokura, Y.
2016-01-01
We have used time-of-flight inelastic neutron scattering to measure the spin wave spectrum of the canonical half-doped manganite Pr0.5Ca0.5MnO3 in its magnetic and orbitally ordered phase. Comparison of the data, which cover multiple Brillouin zones and the entire energy range of the excitations, with several different models shows that only the CE-type ordered state provides an adequate description of the magnetic ground state, provided interactions beyond nearest neighbor are included. We are able to rule out a ground state in which there exist pairs of dimerized spins which interact only with their nearest neighbors. The Zener polaron ground state, whichmore » comprises strongly bound magnetic dimers, can be ruled out on the basis of gross features of the observed spin wave spectrum. A model with weaker dimerization reproduces the observed dispersion but can be ruled out on the basis of subtle discrepancies between the calculated and observed structure factors at certain positions in reciprocal space. Adding further neighbor interactions results in almost no dimerization, i.e. interpolating back to the CE model. These results are consistent with theoretical analysis of the degenerate double exchange model for half-doping.« less
Ewings, Russell A.; Perring, T. G.; Sikora, O.; Abernathy, Douglas L; Tomioka, Y.; Tokura, Y.
2016-01-01
We have used time-of-flight inelastic neutron scattering to measure the spin wave spectrum of the canonical half-doped manganite Pr0.5Ca0.5MnO3 in its magnetic and orbitally ordered phase. Comparison of the data, which cover multiple Brillouin zones and the entire energy range of the excitations, with several different models shows that only the CE-type ordered state provides an adequate description of the magnetic ground state, provided interactions beyond nearest neighbor are included. We are able to rule out a ground state in which there exist pairs of dimerized spins which interact only with their nearest neighbors. The Zener polaron ground state, which comprises strongly bound magnetic dimers, can be ruled out on the basis of gross features of the observed spin wave spectrum. A model with weaker dimerization reproduces the observed dispersion but can be ruled out on the basis of subtle discrepancies between the calculated and observed structure factors at certain positions in reciprocal space. Adding further neighbor interactions results in almost no dimerization, i.e. interpolating back to the CE model. These results are consistent with theoretical analysis of the degenerate double exchange model for half-doping.
NASA Astrophysics Data System (ADS)
Zhou, R.; Xing, L. Y.; Wang, X. C.; Jin, C. Q.; Zheng, Guo-qing
2016-02-01
In copper-oxide and iron-based high-temperature (high-Tc) superconductors, many physical properties exhibit in-plane anisotropy, which is believed to be caused by a rotational symmetry-breaking nematic order, whose origin and its relationship to superconductivity remain elusive. In many iron pnictides, a tetragonal-to-orthorhombic structural transition temperature Ts coincides with the magnetic transition temperature TN, making the orbital and spin degrees of freedom highly entangled. NaFeAs is a system where Ts=54 K is well separated from TN=42 K, which helps simplify the experimental situation. Here we report nuclear magnetic resonance (NMR) measurements on NaFe1 -xCoxAs (0 ≤x ≤0.042 ) that revealed orbital and spin nematicity occurring at a temperature T* far above Ts in the tetragonal phase. We show that the NMR spectra splitting and its evolution can be explained by an incommensurate orbital order that sets in below T* and becomes commensurate below Ts, which brings about the observed spin nematicity.
NASA Astrophysics Data System (ADS)
Li, P. H. Y.; Bishop, R. F.; Campbell, C. E.
2015-01-01
We use the coupled cluster method (CCM) to study the zero-temperature ground-state (GS) properties of a spin-1/2 J1-J2 Heisenberg antiferromagnet on a triangular lattice with competing nearest-neighbor and next-nearest-neighbor exchange couplings J1>0 and J2≡κ J1>0 , respectively, in the window 0 ≤κ <1 . The classical version of the model has a single GS phase transition at κcl=1/8 in this window from a phase with 3-sublattice antiferromagnetic (AFM) 120∘ Néel order for κ <κcl to an infinitely degenerate family of 4-sublattice AFM Néel phases for κ >κcl . This classical accidental degeneracy is lifted by quantum fluctuations, which favor a 2-sublattice AFM striped phase. For the quantum model we work directly in the thermodynamic limit of an infinite number of spins, with no consequent need for any finite-size scaling analysis of our results. We perform high-order CCM calculations within a well-controlled hierarchy of approximations, which we show how to extrapolate to the exact limit. In this way we find results for the case κ =0 of the spin-1/2 model for the GS energy per spin, E /N =-0.5521 (2 ) J1 , and the GS magnetic order parameter, M =0.198 (5 ) (in units where the classical value is Mcl=1/2), which are among the best available. For the spin-1/2 J1-J2 model we find that the classical transition at κ =κcl is split into two quantum phase transitions at κ1c=0.060 (10 ) and κ2c=0.165 (5 ) . The two quasiclassical AFM states (viz., the 120∘ Néel state and the striped state) are found to be the stable GS phases in the regime κ <κ1c and κ >κ2c , respectively, while in the intermediate regimes κ1c<κ <κ2c the stable GS phase has no evident long-range magnetic order.
Mapping spin-wave dispersions in stripe-ordered La2-xSrxNiO4 ( x=0.275 , 0.333)
NASA Astrophysics Data System (ADS)
Woo, Hyungje; Boothroyd, A. T.; Nakajima, K.; Perring, T. G.; Frost, C. D.; Freeman, P. G.; Prabhakaran, D.; Yamada, K.; Tranquada, J. M.
2005-08-01
Using the MAPS spectrometer at the ISIS spallation source, we have measured the magnetic excitations of single-crystal samples of stripe-ordered La2-xSrxNiO4 with x=0.333 and 0.275. The full two-dimensional spin-wave dispersions were obtained using incident energies of 60 and 160 meV. To analyze the excitations, we have evaluated a spin-only Hamiltonian describing diagonal, site-centered stripes in the linear spin-wave approximation. Besides the superexchange energy J within antiferromagnetic domains, we have considered effective exchange couplings J1 and J2 across a charge stripe coupling second-neighbor Ni sites along Ni-O bond directions and along the plaquette diagonal, respectively. From least-squares fits of the model to the measurements on the x=1/3 sample at T=10K , we find that the dispersions are well described by a model using just J and J1 , but not J and J2 . Consistent with an analysis of previous measurements, we find that J is about 90% of the superexchange energy of undoped La2NiO4 and J1/J≈0.5 . The excitations observed for x=0.275 are surprisingly similar to those for x=1/3 , despite the differing magnetic-ordering wave vectors; the main difference is a broadening of the excitations for x=0.275 . For both samples, we find that one spin-wave branch has a gap of ˜20meV , confirming a previous observation for x=1/3 . We discuss the possible origin of this gap.
Kim, Youngjae; Yun, Won Seok; Lee, J D
2016-01-01
Functionalized X-Bi bilayers (X = Ga, In, and Tl) with halogens bonded on their both sides have been recently claimed to be the giant topological insulators due to the strong band inversion strengths. Employing the first-principles electronic structure calculation, we find the topological band order transition from the order p - p - s of the X-Bi bilayers with halogens on their both sides to the new order p - s - p of the bilayers (especially for X = Ga and In) with halogen on one side and hydrogen on the other side, where the asymmetric hydrogen bonding simulates the substrate. We further find that the p - s bulk band gap of the bilayer bearing the new order p - s - p sensitively depends on the electric field, which enables a meaningful engineering of the quantum spin Hall edge state by controlling the external electric field. PMID:27623710
NASA Astrophysics Data System (ADS)
Schönecker, Stephan; Li, Xiaoqing; Johansson, Börje; Vitos, Levente
2016-08-01
The strained Fe-Co alloy in body-centered tetragonal (bct) structure has raised considerable interest due to its giant uniaxial magnetocrystalline anisotropy energy. On the basis of the classical Heisenberg Hamiltonian with ab initio interatomic exchange interactions, we perform a theoretical study of fundamental finite temperature magnetic properties of Fe1 -xCox alloy films as a function of three variables: chemical composition 0.3 ≤x ≤0.8 , bct geometry [a ,c (a )] arising from in-plane strain and associated out-of-plane relaxation, and atomic long-range order (ALRO). The Curie temperatures TC(x ,a ) obtained from Monte Carlo simulations display a competition between a pronounced dependence on tetragonality, strong ferromagnetism in the Co-rich alloy, and the beginning instability of ferromagnetic order in the Fe-rich alloy when c /a →√{2 } . Atomic ordering enhances TC and arises mainly due to different distributions of atoms in neighboring coordination shells rather than altering exchange interactions significantly. We investigate the ordering effect on the shape of the adiabatic spin-wave spectrum for selected pairs (x ,a ) . Our results indicate that long-wavelength acoustic spin-wave excitations show dependencies on x , a , and ALRO similar to those of TC. The directional anisotropy of the spin-wave stiffness d (x ,a ) peaks in narrow ranges of composition and tetragonality. ALRO exhibits a strong effect on d for near equiconcentration Fe-Co. We also discuss our findings in the context of employing Fe-Co as perpendicular magnetic recording medium.
NASA Astrophysics Data System (ADS)
Delgado Acosta, E. G.; Banda Guzmán, V. M.; Kirchbach, M.
2015-03-01
We propose a general method for the description of arbitrary single spin- j states transforming according to ( j, 0) ⊕ (0, j) carrier spaces of the Lorentz algebra in terms of Lorentz tensors for bosons, and tensor-spinors for fermions, and by means of second-order Lagrangians. The method allows to avoid the cumbersome matrix calculus and higher ∂2 j order wave equations inherent to the Weinberg-Joos approach. We start with reducible Lorentz tensor (tensor-spinor) representation spaces hosting one sole ( j, 0) ⊕ (0, j) irreducible sector and design there a representation reduction algorithm based on one of the Casimir invariants of the Lorentz algebra. This algorithm allows us to separate neatly the pure spin- j sector of interest from the rest, while preserving the separate Lorentz and Dirac indexes. However, the Lorentz invariants are momentum independent and do not provide wave equations. Genuine wave equations are obtained by conditioning the Lorentz tensors under consideration to satisfy the Klein-Gordon equation. In so doing, one always ends up with wave equations and associated Lagrangians that are of second order in the momenta. Specifically, a spin-3/2 particle transforming as (3/2, 0) ⊕ (0, 3/2) is comfortably described by a second-order Lagrangian in the basis of the totally anti-symmetric Lorentz tensor-spinor of second rank, Ψ [ μν]. Moreover, the particle is shown to propagate causally within an electromagnetic background. In our study of (3/2, 0) ⊕ (0, 3/2) as part of Ψ [ μν] we reproduce the electromagnetic multipole moments known from the Weinberg-Joos theory. We also find a Compton differential cross-section that satisfies unitarity in forward direction. The suggested tensor calculus presents itself very computer friendly with respect to the symbolic software FeynCalc.
Haidar, S. M. Iguchi, R.; Yagmur, A.; Lustikova, J.; Shiomi, Y.; Saitoh, E.
2015-05-14
We have investigated dc voltage generation induced by ferromagnetic resonance in a Co{sub 75}Fe{sub 25}/Pt film. In order to reduce rectification effects of anisotropic magnetoresistance and the planar Hall effect, which may be observed simultaneously with the inverse spin Hall effect, we selected Co{sub 75}Fe{sub 25} with extremely small anisotropic magnetoresistance as a spin injector. Using the difference in the spectral shape of voltage and in the angle dependence of in-plane magnetization among the effects, we demonstrated that the generated dc voltage is governed by the inverse spin Hall effect induced by spin pumping.
Long-range order and spin-liquid states of polycrystalline Tb2+xTi2-xO7+y
Taniguchi, T; Kadowaki, Hiroaki; Takatsu, Hiroshi; Fak, B; Yamazaki, Teruo; Saito, Tomonori; Yoshizawa, H.; Shimura, Y; Sakakibara, T; Hong, T; Goto, K; Yaraskavitch, L; Kycia, J
2013-01-01
Low-temperature states of polycrystalline samples of a frustrated pyrochlore oxide Tb2+xTi2 xO7+y have been investigated by specific heat, magnetic susceptibility, and neutron scattering experiments. We have found that this system can be tuned by a minute change of x from a spin-liquid state (x < xc) to a partly ordered state with a small antiferromagnetic ordering of the order of 0.1 B. Specific heat shows a sharp peak at a phase transition at Tc = 0.5 K for x = 0.005. Magnetic excitation spectra for this sample change from a quasielastic to a gapped type through Tc. The possibility of a Jahn-Teller transition is discussed.
S. -H. Baek; Gu, G. D.; Utz, Y.; Hucker, M.; Buchner, B.; Grafe, H. -J.
2015-10-26
We report ^{139}La nuclear magnetic resonance studies performed on a La_{1.875}Ba_{0.125}CuO_{4} single crystal. The data show that the structural phase transitions (high-temperature tetragonal → low-temperature orthorhombic → low-temperature tetragonal phase) are of the displacive type in this material. The ^{139}La spin-lattice relaxation rate T^{–1}_{1} sharply upturns at the charge-ordering temperature T_{CO} = 54 K, indicating that charge order triggers the slowing down of spin fluctuations. Detailed temperature and field dependencies of the T^{–1}_{1} below the spin-ordering temperature T_{SO}=40 K reveal the development of enhanced spin fluctuations in the spin-ordered state for H ∥ [001], which are completely suppressed for large fields along the CuO_{2} planes. Lastly, our results shed light on the unusual spin fluctuations in the charge and spin stripe ordered lanthanum cuprates.
Spin dynamics, short-range order, and spin freezing in Y{sub 0.5}Ca{sub 0.5}BaCo{sub 4}O{sub 7}
Stewart, J. R.; Ehlers, G.; Mutka, H.; Fouquet, P.; Payen, C.; Lortz, R.
2011-01-15
Y{sub 0.5}Ca{sub 0.5}BaCo{sub 4}O{sub 7} was recently introduced as a possible candidate for capturing some of the predicted classical spin kagome ground-state features. Stimulated by this conjecture, we have taken up a more complete study of the spin correlations in this compound with neutron scattering methods on a powder sample characterized with high-resolution neutron diffraction and the temperature dependence of magnetic susceptibility and specific heat. We have found that the frustrated near-neighbor magnetic correlations involve not only the kagome planes but concern the full Co sublattice, as evidenced by the analysis of the wave-vector dependence of the short-range order. We conclude from our results that the magnetic moments are located on the Co sublattice as a whole and that correlations extend beyond the two-dimensional kagome planes. We identify intriguing dynamical properties, observing high-frequency fluctuations with a Lorentzian linewidth {Gamma}{<=}20 meV at ambient temperature. On cooling a low-frequency ({approx}1 meV) dynamical component develops alongside the high-frequency fluctuations, which eventually becomes static at temperatures below T{approx_equal}50 K. The high-frequency response with an overall linewidth of {approx}10 meV prevails at T{<=}2 K, coincident with a fully elastic short-range-ordered contribution.
Spin relaxation through Kondo scattering in Cu/Py lateral spin valves
NASA Astrophysics Data System (ADS)
Batley, J. T.; Rosaond, M. C.; Ali, M.; Linfield, E. H.; Burnell, G.; Hickey, B. J.
Within non-magnetic metals it is reasonable to expect the Elliot-Yafet mechanism to govern spin-relaxation and thus the temperature dependence of the spin diffusion length might be inversely proportional to resistivity. However, in lateral spin valves, measurements have found that at low temperatures the spin diffusion length unexpectedly decreases. We have fabricated lateral spin valves from Cu with different concentrations of magnetic impurities. Through temperature dependent charge and spin transport measurements we present clear evidence linking the presence of the Kondo effect within Cu to the suppression of the spin diffusion length below 30 K. We have calculated the spin-relaxation rate and isolated the contribution from magnetic impurities. At very low temperatures electron-electron interactions play a more prominent role in the Kondo effect. Well below the Kondo temperature a strong-coupling regime exists, where the moments become screened and the magnetic dephasing rate is reduced. We also investigate the effect of this low temperature regime (>1 K) on a pure spin current. This work shows the dominant role of Kondo scattering, even in low concentrations of order 1 ppm, within pure spin transport.
Śmiga, Szymon; Della Sala, Fabio; Buksztel, Adam; Grabowski, Ireneusz; Fabiano, Eduardo
2016-08-15
One important property of Kohn-Sham (KS) density functional theory is the exact equality of the energy of the highest occupied KS orbital (HOMO) with the negative ionization potential of the system. This exact feature is out of reach for standard density-dependent semilocal functionals. Conversely, accurate results can be obtained using orbital-dependent functionals in the optimized effective potential (OEP) approach. In this article, we investigate the performance, in this context, of some advanced OEP methods, with special emphasis on the recently proposed scaled-opposite-spin OEP functional. Moreover, we analyze the impact of the so-called HOMO condition on the final quality of the HOMO energy. Results are compared to reference data obtained at the CCSD(T) level of theory. © 2016 Wiley Periodicals, Inc. PMID:27357413
Spin noise in mixed Spin Systems
NASA Astrophysics Data System (ADS)
Bauch, Erik; Junghyun, Paul; Singh, Swati; Devakul, Trithep; Feguin, Adrian; Hart, Connor; Walsworth, Ronald
2016-05-01
The spin noise due to interaction of multiple spin species in mixed spin systems provides a fundamental limit to ultra-sensitive ensemble sensing and quantum information applications. In our work, we investigate the interaction of dense nuclear 13C spins with electronic nitrogen spins using Nitrogen-Vacancy centers in diamond. Our work shows experimentally and theoretically, that under certain conditions, spin noise is greatly suppressed and the coherence time of NV centers improved by order of magnitudes, providing a pathway to engineering high density ensemble samples with long coherence times at room temperature.
NASA Astrophysics Data System (ADS)
Liu, Jin Hua; Wang, Hai Tao
2015-10-01
Topological quantum phase transitions are numerically investigated in a spin-1/2 dimerized and frustrated Heisenberg chain by using infinite matrix product state representation with the infinite time evolving block decimation method. Quantum fidelity approach is employed to detect the degenerate ground states and quantum phase transitions. By calculating the long-range string order parameters, we find two topological Haldane phases characterized by two long-range string orders. Also, continuous and discontinuous behaviors of von Neumann entropy show that phase transitions between two topological Haldane phases are topologically continuous and discontinuous quantum phase transitions. For the topologically continuous phase transition, the central charge at the critical point is obtained as c = 1, which means that the topologically continuous quantum phase transition belongs to the Gaussian universality class.
Spin frustration and magnetic ordering in triangular lattice antiferromagnet Ca3CoNb2O9
NASA Astrophysics Data System (ADS)
Dai, Jia; Zhou, Ping; Wang, Peng-Shuai; Pang, Fei; Munsie, Tim J.; Luke, Graeme M.; Zhang, Jin-Shan; Yu, Wei-Qiang
2015-12-01
We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca3CoNb2O9, in which the effective spin of Co2+ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and magnetization techniques. The x-ray diffraction confirms the quality of our powder samples. The large Weiss constant θCW˜ -55 K and the low Neel temperature TN˜ 1.45 K give a frustration factor f = | θCW/TN | ≈ 38, suggesting that Ca3CoNb2O9 resides in strong frustration regime. Slightly below TN, deviation between the susceptibility data under zero-field cooling (ZFC) and field cooling (FC) is observed. A new magnetic state with 1/3 of the saturate magnetization Ms is suggested in the magnetization curve at 0.46 K. Our study indicates that Ca3CoNb2O9 is an interesting material to investigate magnetism in triangular lattice antiferromagnets with weak anisotropy. Project supported by the National Natural Science Foundation of China (Grant Nos. 11374364 and 11222433), the National Basic Research Program of China (Grant No. 2011CBA00112). Research at McMaster University supported by the Natural Sciences and Engineering Research Council. Work at North China Electric Power University supported by the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry.
Nematic order in a simple-cubic lattice-spin model with full-ranged dipolar interactions
NASA Astrophysics Data System (ADS)
Chamati, Hassan; Romano, Silvano
2016-05-01
In a previous paper [Phys. Rev. E 90, 022506 (2014), 10.1103/PhysRevE.90.022506], we studied the thermodynamic and structural properties of a three-dimensional simple-cubic lattice model with dipolarlike interaction, truncated at nearest-neighbor separation, for which the existence of an ordering transition at finite temperature had been proven mathematically; here we extend our investigation, addressing the full-ranged counterpart of the model, for which the critical behavior had been investigated theoretically and experimentally. In addition, the existence of an ordering transition at finite temperature had been proven mathematically as well. Both models exhibited the same continuously degenerate ground-state configuration, possessing full orientational order with respect to a suitably defined staggered magnetization (polarization), but no nematic second-rank order; in both cases, thermal fluctuations remove the degeneracy, so that nematic order does set in at low but finite temperature via a mechanism of order by disorder. On the other hand, there were recognizable quantitative differences between the two models as for ground-state energy and critical exponent estimates; the latter were found to agree with early renormalization-group calculations and with experimental results.
Nematic order in a simple-cubic lattice-spin model with full-ranged dipolar interactions.
Chamati, Hassan; Romano, Silvano
2016-05-01
In a previous paper [Phys. Rev. E 90, 022506 (2014)PLEEE81539-375510.1103/PhysRevE.90.022506], we studied the thermodynamic and structural properties of a three-dimensional simple-cubic lattice model with dipolarlike interaction, truncated at nearest-neighbor separation, for which the existence of an ordering transition at finite temperature had been proven mathematically; here we extend our investigation, addressing the full-ranged counterpart of the model, for which the critical behavior had been investigated theoretically and experimentally. In addition, the existence of an ordering transition at finite temperature had been proven mathematically as well. Both models exhibited the same continuously degenerate ground-state configuration, possessing full orientational order with respect to a suitably defined staggered magnetization (polarization), but no nematic second-rank order; in both cases, thermal fluctuations remove the degeneracy, so that nematic order does set in at low but finite temperature via a mechanism of order by disorder. On the other hand, there were recognizable quantitative differences between the two models as for ground-state energy and critical exponent estimates; the latter were found to agree with early renormalization-group calculations and with experimental results. PMID:27300869
Thompson, Corey; Greedan, John; Garlea, Vasile O; Flacau, Roxana; Tan, Malinda; Derakhshan, Shahab
2014-01-01
The novel iron-based compound, BaYFeO4, crystallizes in the Pnma space group with two distinct Fe3+ sites, that are alternately corner-shared [FeO5]7 square pyramids and [FeO6]9 octahedra, forming into [Fe4O18]24 rings, which propagate as columns along the b-axis. A recent report shows two discernible antiferromagnetic (AFM) transitions at 36 and 48 K in the susceptibility, yet heat capacity measurements reveal no magnetic phase transitions at these temperatures. An upturn in the magnetic susceptibility measurements up to 400 K suggests the presence of shortrange magnetic behavior at higher temperatures. In this Article, variable-temperature neutron powder diffraction and hightemperature magnetic susceptibility measurements were performed to clarify the magnetic behavior. Neutron powder diffraction confirmed that the two magnetic transitions observed at 36 and 48 K are due to long-range magnetic order. Below 48 K, the magnetic structure was determined as a spin-density wave (SDW) with a propagation vector, k = (0, 0, 1/3), and the moments along the b-axis, whereas the structure becomes an incommensurate cycloid [k = (0, 0, 0.35)] below 36 K with the moments within the bc-plane. However, for both cases the ordered moments on Fe3+ are only of the order 3.0 B, smaller than the expected values near 4.5 B, indicating that significant components of the Fe moments remain paramagnetic to the lowest temperature studied, 6 K. Moreover, new high-temperature magnetic susceptibility measurements revealed a peak maximum at 550 K indicative of short-range spin correlations. It is postulated that most of the magnetic entropy is thus removed at high temperatures which could explain the absence of heat capacity anomalies at the long-range ordering temperatures. Published spin dimer calculations, which appear to suggest a k = (0, 0, 0) magnetic structure, and allow for neither low dimensionality nor geometric frustration, are inadequate to explain the observed complex magnetic
NASA Astrophysics Data System (ADS)
Taghavi-Shahri, F.; Khanpour, Hamzeh; Atashbar Tehrani, S.; Alizadeh Yazdi, Z.
2016-06-01
We present a first QCD analysis of next-to-next-leading-order (NNLO) contributions of the spin-dependent parton distribution functions (PPDFs) in the nucleon and their uncertainties using the Jacobi polynomial approach. Having the NNLO contributions of the quark-quark and gluon-quark splitting functions in perturbative QCD [Nucl. Phys. B889, 351 (2014)], one can obtain the evolution of longitudinally polarized parton densities of hadrons up to NNLO accuracy of QCD. Very large sets of recent and up-to-date experimental data of spin structure functions of the proton g1p, neutron g1n, and deuteron g1d have been used in this analysis. The predictions for the NNLO calculations of the polarized parton distribution functions as well as the proton, neutron and deuteron polarized structure functions are compared with the corresponding results of the NLO approximation. We form a mutually consistent set of polarized PDFs due to the inclusion of the most available experimental data including the recently high-precision measurements from COMPASS16 experiments [Phys. Lett. B 753, 18 (2016)]. We have performed a careful estimation of the uncertainties using the most common and practical method, the Hessian method, for the polarized PDFs originating from the experimental errors. The proton, neutron and deuteron structure functions and also their first moments, Γp ,n ,d , are in good agreement with the experimental data at small and large momentum fractions of x . We will discuss how our knowledge of spin-dependence structure functions can improve at small and large values of x by the recent COMPASS16 measurements at CERN, the PHENIX and STAR measurements at RHIC, and at the future proposed colliders such as the Electron-Ion Collider.
NASA Astrophysics Data System (ADS)
Shah, Abhay G.; Pound, Adam
2015-06-01
Using black hole perturbation theory and arbitrary-precision computer algebra, we obtain the post-Newtonian expansions of the linear-in-mass-ratio corrections to the spin-precession angle and tidal invariants for a particle in circular orbit around a Schwarzschild black hole. We extract coefficients up to 20 post-Newtonian order from numerical results that are calculated with an accuracy greater than 1 part in 10500. These results can be used to calibrate parameters in effective-one-body models of compact binaries, specifically the spin-orbit part of the effective Hamiltonian and the dynamically significant tidal part of the main radial potential of the effective metric. Our calculations are performed in a radiation gauge, which is known to be singular away from the particle. To overcome this irregularity, we define suitable Detweiler-Whiting singular and regular fields in this gauge, and we compute the invariants using mode-sum regularization in combination with averaging from two sides of the particle. The detailed justification of this regularization procedure will be presented in a forthcoming companion paper.
NASA Astrophysics Data System (ADS)
Kato, Hatsuhiro; Kato, Hatsuyoshi
2016-05-01
We proposed a new discretisation scheme for deriving a second-order difference equation from any system being formulated with the weak-form theory framework. The proposed scheme enables us to extend the application range of the recursive transfer method (RTM) and to express perfectly matching conditions for port boundaries in a discrete fashion under the RTM framework. To evaluate the accuracy and demonstrate the validity of the proposed scheme, we discussed the scattering problem governed by the fourth-order differential equation that was hitherto outside the RTM application range. The difference equation can play an important role in maintaining the balance of the bending moment and the shear force at the interface of two segments. Using the new port boundary condition, a quasi-localised wave was extracted and found to be related to the phase shift due to Fano resonance.
Ferromagnetic ordering of minority Ce3 + spins in a quasi-skutterudite Ce 3Os 4Ge13 single crystal
NASA Astrophysics Data System (ADS)
Prakash, Om; Thamizhavel, A.; Ramakrishnan, S.
2016-02-01
We report site disorder driven ferromagnetic ordering of nearly 8 % Ce atoms in single crystalline Ce 3Os 4Ge13 below 0.5 K. Ce 3Os 4Ge13 crystallizes in a cubic structure with space group Pm 3 ¯n . The structural analysis shows the presence of site disorder in the system, where the 2 (a ) Ge site is partially occupied by the Ce atoms. Due to the small Ce 4 f -ligand hybridization, these Ce atoms are in the Ce3 + (magnetic) state while the rest of the Ce atoms in the unit cell are in the Ce4 -δ (nonmagnetic) state. The heat capacity shows a peak below 0.5 K corresponding to the ferromagnetic ordering of the Ce3 + moments. The ferromagnetic ordering below 0.5 K is also seen in the ac-susceptibility data. At low temperatures (1.8 K ≤T ≤6 K), the magnetization shows ln (T ) dependence, whereas the resistivity shows power-law (Tn) temperature dependence indicating the non-Fermi-liquid behavior of the quasiparticles.
Lefrancois, Daniel; Rehn, Dirk R; Dreuw, Andreas
2016-08-28
For the calculation of adiabatic singlet-triplet gaps (STG) in diradicaloid systems the spin-flip (SF) variant of the algebraic diagrammatic construction (ADC) scheme for the polarization propagator in third order perturbation theory (SF-ADC(3)) has been applied. Due to the methodology of the SF approach the singlet and triplet states are treated on an equal footing since they are part of the same determinant subspace. This leads to a systematically more accurate description of, e.g., diradicaloid systems than with the corresponding non-SF single-reference methods. Furthermore, using analytical excited state gradients at ADC(3) level, geometry optimizations of the singlet and triplet states were performed leading to a fully consistent description of the systems, leading to only small errors in the calculated STGs ranging between 0.6 and 2.4 kcal/mol with respect to experimental references. PMID:27586899
Luo, Alan M; Wenk, Stefan; Ilg, Patrick
2015-04-01
In Romano's Comment [Phys. Rev. E 91, 046501 (2015)] on Sec. II of our paper [Phys. Rev. E 90, 022502 (2014)], the author suggests that our findings concerning the nature of the ordering transition of our modified Lebwohl-Lasher model with two-dimensional planar rotators on a planar lattice are inconsistent with known mathematical results. We argue in this Reply that our findings are in fact in agreement with previous mathematical and simulation results and that the criticisms raised by Romano have no impact on the results presented in our paper. PMID:25974614
All-in-all-Out Magnetic Order and Propagating Spin Waves in Sm2Ir2O7
NASA Astrophysics Data System (ADS)
Donnerer, C.; Rahn, M. C.; Sala, M. Moretti; Vale, J. G.; Pincini, D.; Strempfer, J.; Krisch, M.; Prabhakaran, D.; Boothroyd, A. T.; McMorrow, D. F.
2016-07-01
Using resonant magnetic x-ray scattering we address the unresolved nature of the magnetic ground state and the low-energy effective Hamiltonian of Sm2 Ir2 O7 , a prototypical pyrochlore iridate with a finite temperature metal-insulator transition. Through a combination of elastic and inelastic measurements, we show that the magnetic ground state is an all-in-all-out (AIAO) antiferromagnet. The magnon dispersion indicates significant electronic correlations and can be well described by a minimal Hamiltonian that includes Heisenberg exchange [J =27.3 (6 ) meV ] and Dzyaloshinskii-Moriya interactions [D =4.9 (3 ) meV ], which provides a consistent description of the magnetic order and excitations. In establishing that Sm2 Ir2 O7 has the requisite inversion symmetry preserving AIAO magnetic ground state, our results support the notion that pyrochlore iridates may host correlated Weyl semimetals.
All-in-all-Out Magnetic Order and Propagating Spin Waves in Sm_{2}Ir_{2}O_{7}.
Donnerer, C; Rahn, M C; Sala, M Moretti; Vale, J G; Pincini, D; Strempfer, J; Krisch, M; Prabhakaran, D; Boothroyd, A T; McMorrow, D F
2016-07-15
Using resonant magnetic x-ray scattering we address the unresolved nature of the magnetic ground state and the low-energy effective Hamiltonian of Sm_{2}Ir_{2}O_{7}, a prototypical pyrochlore iridate with a finite temperature metal-insulator transition. Through a combination of elastic and inelastic measurements, we show that the magnetic ground state is an all-in-all-out (AIAO) antiferromagnet. The magnon dispersion indicates significant electronic correlations and can be well described by a minimal Hamiltonian that includes Heisenberg exchange [J=27.3(6) meV] and Dzyaloshinskii-Moriya interactions [D=4.9(3) meV], which provides a consistent description of the magnetic order and excitations. In establishing that Sm_{2}Ir_{2}O_{7} has the requisite inversion symmetry preserving AIAO magnetic ground state, our results support the notion that pyrochlore iridates may host correlated Weyl semimetals. PMID:27472131
Influence of interstitial Mn on spin order and dynamics in the room-temperature ferromagnet Mn1+δSb
NASA Astrophysics Data System (ADS)
Taylor, Alice
Mn1+δSb is a well-known, high Curie temperature, ferromagnetic metal. It has particular importance because it, and closely related MnBi, show promise as alternatives to rare-earth-containing permanent magnets, and as magneto-optic media. To exploit these materials' useful properties, it is desirable to tune and optimize the magnetic properties. To achieve this, the magnetic interactions, and the effects of doping and defects must be understood. In Mn1+δSb the magnetic order is highly sensitive to the interstitial Mn ion content, δ, suggesting a route to tune the properties. However, detailed theoretical and experimental investigations of the effect of the interstitial ion, Mn2, have been lacking, probably due to a prevailing view in the literature that the Mn2 site is nonmagnetic. We examine the magnetic state of Mn2, and its influence on the magnetic properties of Mn1+δSb. We use a combination of neutron scattering techniques alongside detailed calculations to show that the Mn2 site is in-fact magnetic, and has a dramatic impact on the magnetic dynamics in Mn1+δSb. An unusual, broad, intense feature is identified in the magnetic dynamics which cannot be explained by the long-range symmetry of the material. This reveals an area in which current theoretical/modeling techniques limit our ability to understand the magnetic excitations revealed by neutron scattering. This investigation elucidates important aspects of the behavior of Mn1+δSb, whilst highlighting requirements for future research to understand the major influence of the interstitial ion on the magnetic properties.
Magneto-anisotropy of spin dephasing in a [001]-grown high-mobility two-dimensional electron system
NASA Astrophysics Data System (ADS)
Korn, T.; Stich, D.; Schulz, R.; Schuh, D.; Wegscheider, W.; Schüller, C.
2010-01-01
The spin dynamics in [001]-grown two-dimensional electron systems (2DES) at low temperatures are governed by the effective spin-orbit fields, which lead to dephasing via the D'yakonov-Perel mechanism. If both the Rashba and the Dresselhaus spin-orbit fields are present and of the same order, their interference causes a large anisotropy of the spin dephasing times for spin orientation along different in-plane directions. This may be observed in time-resolved Faraday rotation measurements using in-plane magnetic fields. The dephasing anisotropy is strongly reduced for increasing carrier density by the increasing importance of the kubic Dresselhaus term.
Charge ordering in NaV_2O_5: INS of the spin dynamics and X-ray anomalous scattering studies.
NASA Astrophysics Data System (ADS)
Grenier, Beatrice
2002-03-01
At room temperature, NaV_2O5 is well described by a quarter-filled two-leg ladder system, with only one type of vanadium site V^4.5+, spins 1/2 being delocalized on the V-O-V rungs. Interestingly, NaV_2O5 undergoes a phase transition at T_c~= 34 K associated to 1/ a lattice distorsion leading to a large unit cell (2a.2b.4c), 2/ the opening of a finite energy gap to the lowest triplet state, 3/ a charge ordering with two types of vanadium sites, V^4.5+δ and V^4.5-δ. But the 3D configuration of the charge ordering is still under debate. The aim of this paper is the determination of the electronic re-distribution occuring below Tc using two complementary techniques. Inelastic neutron scattering results are first presented.^1 Spin excitations have been studied along the two directions (Q_a,1/2,0) and (Q_a,1,0). Two branches with distinct energy gaps are identified, with a weak dispersion along Qa (δ J ~= 1 meV along the ladder rungs), reflecting the low dimensionality of the magnetic interactions (Jb ~= 60 meV along the ladder legs). From the dispersion and the analysis of the structure factors, the 2D charge distribution is deduced in the (a,b) planes: the experimental data agree well with a zig-zag charge distribution on the ladder rungs and lead to a charge transfer amounting δ = 0.3. An X-ray anomalous scattering study, performed on the K-edge of the vanadium atom, is then discussed.^2 A large number of Bragg reflections from both phases has been measured as a function of the incident photon energy. The data confirm the zig-zag picture issued from INS, with a smaller charge transfer, and the 3D charge order arrangement is found to be rather complex. It suggests stacking faults separating regions corresponding to four possible patterns. In the light of these X-ray results, our neutron data are further analyzed. ^1B. Grenier et al., Phys. Rev. Lett. 86 (2001) 5966. ^2S. Grenier et al., cond-mat/0109091.
NASA Astrophysics Data System (ADS)
Adolph, C.; Alekseev, M. G.; Alexakhin, V. Yu.; Alexandrov, Yu.; Alexeev, G. D.; Amoroso, A.; Antonov, A. A.; Austregesilo, A.; Badełek, B.; Balestra, F.; Barth, J.; Baum, G.; Bedfer, Y.; Berlin, A.; Bernhard, J.; Bertini, R.; Bettinelli, M.; Bicker, K.; Bieling, J.; Birsa, R.; Bisplinghoff, J.; Bordalo, P.; Bradamante, F.; Braun, C.; Bravar, A.; Bressan, A.; Büchele, M.; Burtin, E.; Capozza, L.; Chiosso, M.; Chung, S. U.; Cicuttin, A.; Crespo, M. L.; Dalla Torre, S.; Das, S.; Dasgupta, S. S.; Dasgupta, S.; Denisov, O. Yu.; Dhara, L.; Donskov, S. V.; Doshita, N.; Duic, V.; Dünnweber, W.; Dziewiecki, M.; Efremov, A.; Elia, C.; Eversheim, P. D.; Eyrich, W.; Faessler, M.; Ferrero, A.; Filin, A.; Finger, M.; Finger, M., Jr.; Fischer, H.; Franco, C.; du Fresne von Hohenesche, N.; Friedrich, J. M.; Frolov, V.; Garfagnini, R.; Gautheron, F.; Gavrichtchouk, O. P.; Gerassimov, S.; Geyer, R.; Giorgi, M.; Gnesi, I.; Gobbo, B.; Goertz, S.; Grabmüller, S.; Grasso, A.; Grube, B.; Gushterski, R.; Guskov, A.; Guthörl, T.; Haas, F.; von Harrach, D.; Heinsius, F. H.; Herrmann, F.; Heß, C.; Hinterberger, F.; Horikawa, N.; Höppner, Ch.; d'Hose, N.; Huber, S.; Ishimoto, S.; Ivanov, O.; Ivanshin, Yu.; Iwata, T.; Jahn, R.; Jary, V.; Jasinski, P.; Joosten, R.; Kabuß, E.; Kang, D.; Ketzer, B.; Khaustov, G. V.; Khokhlov, Yu. A.; Kisselev, Yu.; Klein, F.; Klimaszewski, K.; Koblitz, S.; Koivuniemi, J. H.; Kolosov, V. N.; Kondo, K.; Königsmann, K.; Konorov, I.; Konstantinov, V. F.; Korzenev, A.; Kotzinian, A. M.; Kouznetsov, O.; Krämer, M.; Kroumchtein, Z. V.; Kunne, F.; Kurek, K.; Lauser, L.; Lednev, A. A.; Lehmann, A.; Levorato, S.; Lichtenstadt, J.; Liska, T.; Maggiora, A.; Magnon, A.; Makke, N.; Mallot, G. K.; Mann, A.; Marchand, C.; Martin, A.; Marzec, J.; Matsuda, T.; Meshcheryakov, G.; Meyer, W.; Michigami, T.; Mikhailov, Yu. V.; Morreale, A.; Mutter, A.; Nagaytsev, A.; Nagel, T.; Nerling, F.; Neubert, S.; Neyret, D.; Nikolaenko, V. I.; Nowak, W.-D.; Nunes, A. S.; Olshevsky, A. G.; Ostrick, M.; Padee, A.; Panknin, R.; Panzieri, D.; Parsamyan, B.; Paul, S.; Perevalova, E.; Pesaro, G.; Peshekhonov, D. V.; Piragino, G.; Platchkov, S.; Pochodzalla, J.; Polak, J.; Polyakov, V. A.; Pretz, J.; Quaresma, M.; Quintans, C.; Rajotte, J.-F.; Ramos, S.; Rapatsky, V.; Reicherz, G.; Rocco, E.; Rondio, E.; Rossiyskaya, N. S.; Ryabchikov, D. I.; Samoylenko, V. D.; Sandacz, A.; Sapozhnikov, M. G.; Sarkar, S.; Savin, I. A.; Sbrizzai, G.; Schiavon, P.; Schill, C.; Schlüter, T.; Schmidt, A.; Schmidt, K.; Schmitt, L.; Schmïden, H.; Schönning, K.; Schopferer, S.; Schott, M.; Shevchenko, O. Yu.; Silva, L.; Sinha, L.; Sissakian, A. N.; Slunecka, M.; Smirnov, G. I.; Sosio, S.; Sozzi, F.; Srnka, A.; Steiger, L.; Stolarski, M.; Sulc, M.; Sulej, R.; Suzuki, H.; Sznajder, P.; Takekawa, S.; Ter Wolbeek, J.; Tessaro, S.; Tessarotto, F.; Tkatchev, L. G.; Uhl, S.; Uman, I.; Vandenbroucke, M.; Virius, M.; Vlassov, N. V.; Wang, L.; Weisrock, T.; Wilfert, M.; Windmolders, R.; Wiślicki, W.; Wollny, H.; Zaremba, K.; Zavertyaev, M.; Zemlyanichkina, E.; Ziembicki, M.; Zhuravlev, N.; Zvyagin, A.
2013-03-01
The gluon polarization in the nucleon was measured using open charm production by scattering 160GeV/c polarized muons off longitudinally polarized protons or deuterons. The data were taken by the COMPASS Collaboration between 2002 and 2007. A detailed account is given of the analysis method that includes the application of neural networks. Several decay channels of D0 mesons are investigated. Longitudinal spin asymmetries of the D meson production cross sections are extracted in bins of D0 transverse momentum and energy. At leading order QCD accuracy, the average gluon polarization is determined as ⟨Δg/g⟩LO=-0.06±0.21(stat.)±0.08(syst.) at the scale ⟨μ2⟩≈13(GeV/c)2 and an average gluon momentum fraction ⟨x⟩≈0.11. The average gluon polarization is also obtained at next-to-leading order QCD accuracy as ⟨Δg/g⟩ NLO=-0.13±0.15(stat.)±0.15(syst.) at the scale ⟨μ2⟩≈13(GeV/c)2 and ⟨x⟩≈0.20.
Gomez Sal, J.C.; Garcia Soldevilla, J.; Blanco, J.A.; Espeso, J.I.; Rodriguez Fernandez, J.; Luis, F.; Bartolome, F.; Bartolome, J.
1997-11-01
The low-temperature magnetic and transport properties of the orthorhombic CeNi{sub 0.4}Cu{sub 0.6} compound have been determined from the analysis of specific heat, ac magnetic susceptibility, electrical resistivity, elastic and inelastic neutron scattering. These measurements present intriguing experimental results that could not be explained within the usual phenomenology of Ce-based compounds. C{sub p} and {chi}{sub ac} present anomalies around 1 K corresponding to ferromagnetic order as confirmed by neutron diffraction. The magnetic structure is collinear with very reduced moments, 0.6{mu}{sub B}/Ce lying in the b direction. Additionally, a clear Kondo behavior is observed with a Kondo temperature T{sub K}=1.9K estimated from quasielastic neutron scattering. Above the ordering temperature, further anomalies are observed in C{sub p} and {chi}{sub ac} that could not be explained as originating from crystal electric field or Kondo effects. From the frequency and field dependence of the {chi}{sub ac}, above T{sub c}, a spin-glass state with a freezing temperature T{sub f}=2K is proposed for this compound. This unusual magnetic behavior is discussed in terms of mixed (positive and negative) Ruderman-Kittel-Kasuya-Yosida interactions, randomness (structural disorder), large hybridization (Kondo effect), and strong magnetocrystalline anisotropy (crystal electric field effects). {copyright} {ital 1997} {ital The American Physical Society}
Larsen, Flemming H
2007-04-01
By numerical simulations MAS and QCPMG methods for acquiring spectra of spin-1 nuclei were compared in order to determine the most sensitive experiment for analysis of molecular dynamics. To comply with the large quadrupolar constants for 14N and the CSA reported for 6Li both of these interactions are included up to second order. For 2H and 6Li both QCPMG and single-pulse MAS experiments were suitable for dynamics studies whereas the single-pulse MAS experiment were the method of choice for investigation of 14N dynamics for C(Q)'s larger than 750kHz at 14.1T. This property prohibits excitation of the 14N lineshape using either single hard or softer composite rf-pulses. Focusing on 14N it was demonstrated that the centerband lineshape is sensitive toward both off-MAS and CSA effects. In addition, excitation by real-time pulses showed that proper lineshapes corresponding to a site with a C(Q) of 3MHz may be excited by a very short pulse. PMID:17418539
Arora, Priya; Moudgil, R. K.; Bhukal, Nisha
2015-05-15
Static density-density correlation function has been calculated for a spin-polarized two-dimensional quantum electron fluid by including the first-order exchange and self-energy corrections to the random-phase approximation (RPA). This is achieved by determining these corrections to the RPA linear density-density response function, obtained by solving the equation of motion for the single-particle Green’s function. Resulting infinite hierarchy of equations (involving higher-order Green’s functions) is truncated by factorizing the two-particle Green’s function as a product of the single-particle Green’s function and one-particle distribution function. Numerical results of correlation function are compared directly against the quantum Monte Carlo simulation data due to Tanatar and Ceperley for different coupling parameter (r{sub s}) values. We find almost exact agreement for r{sub s}=1, with a noticeable improvement over the RPA. Its quality, however, deteriorates with increasing r{sub s}, but correction to RPA is quite significant.
NASA Astrophysics Data System (ADS)
Izsák, Róbert; Neese, Frank
2013-07-01
The 'chain of spheres' approximation, developed earlier for the efficient evaluation of the self-consistent field exchange term, is introduced here into the evaluation of the external exchange term of higher order correlation methods. Its performance is studied in the specific case of the spin-component-scaled third-order Møller--Plesset perturbation (SCS-MP3) theory. The results indicate that the approximation performs excellently in terms of both computer time and achievable accuracy. Significant speedups over a conventional method are obtained for larger systems and basis sets. Owing to this development, SCS-MP3 calculations on molecules of the size of penicillin (42 atoms) with a polarised triple-zeta basis set can be performed in ∼3 hours using 16 cores of an Intel Xeon E7-8837 processor with a 2.67 GHz clock speed, which represents a speedup by a factor of 8-9 compared to the previously most efficient algorithm. Thus, the increased accuracy offered by SCS-MP3 can now be explored for at least medium-sized molecules.
Spin-Spin Coupling in Asteroidal Binaries
NASA Astrophysics Data System (ADS)
Batygin, Konstantin; Morbidelli, Alessandro
2015-11-01
Gravitationally bound binaries constitute a substantial fraction of the small body population of the solar system, and characterization of their rotational states is instrumental to understanding their formation and dynamical evolution. Unlike planets, numerous small bodies can maintain a perpetual aspheroidal shape, giving rise to a richer array of non-trivial gravitational dynamics. In this work, we explore the rotational evolution of triaxial satellites that orbit permanently deformed central objects, with specific emphasis on quadrupole-quadrupole interactions. Our analysis shows that in addition to conventional spin-orbit resonances, both prograde and retrograde spin-spin resonances naturally arise for closely orbiting, highly deformed bodies. Application of our results to the illustrative examples of (87) Sylvia and (216) Kleopatra multi-asteroid systems implies capture probabilities slightly below ~10% for leading-order spin-spin resonances. Cumulatively, our results suggest that spin-spin coupling may be consequential for highly elongated, tightly orbiting binary objects.
Spin-liquid condensate of spinful bosons.
Lian, Biao; Zhang, Shoucheng
2014-08-22
We introduce the concept of a bosonic spin liquid condensate (SLC), where spinful bosons in a lattice form a zero-temperature spin disordered charge condensate that preserves the spin rotation symmetry, but breaks the U(1) symmetry due to a spinless order parameter with charge one. It has an energy gap to all the spin excitations. We show that such SLC states can be realized in a system of spin S ≥ 2 bosons. In particular, we analyze the SLC phase diagram in the spin 2 case using a mean-field variational wave function method. We show there is a direct analogy between the SLC and the resonating-valence-bond state. PMID:25192078
The spin-temperature theory of dynamic nuclear polarization and nuclear spin-lattice relaxation
NASA Technical Reports Server (NTRS)
Byvik, C. E.; Wollan, D. S.
1974-01-01
A detailed derivation of the equations governing dynamic nuclear polarization (DNP) and nuclear spin lattice relaxation by use of the spin temperature theory has been carried to second order in a perturbation expansion of the density matrix. Nuclear spin diffusion in the rapid diffusion limit and the effects of the coupling of the electron dipole-dipole reservoir (EDDR) with the nuclear spins are incorporated. The complete expression for the dynamic nuclear polarization has been derived and then examined in detail for the limit of well resolved solid effect transitions. Exactly at the solid effect transition peaks, the conventional solid-effect DNP results are obtained, but with EDDR effects on the nuclear relaxation and DNP leakage factor included. Explicit EDDR contributions to DNP are discussed, and a new DNP effect is predicted.
NASA Astrophysics Data System (ADS)
Calvo, Rafael; Sartoris, Rosana P.; Calvo, Hernán L.; Chagas, Edson F.; Rapp, Raul E.
2016-05-01
We study the spin chain behavior, a transition to 3D magnetic order and the magnitudes of the exchange interactions for the metal-amino acid complex Cu(D,L-alanine)2•H2O, a model compound to investigate exchange couplings supported by chemical paths characteristic of biomolecules. Thermal and magnetic data were obtained as a function of temperature (T) and magnetic field (B0). The magnetic contribution to the specific heat, measured between 0.48 and 30 K, displays above 1.8 K a 1D spin-chain behavior that can be fitted with an intrachain antiferromagnetic (AFM) exchange coupling constant 2J0=(-2.12±0.08) cm-1 (defined as ℋex(i,i+1) = -2J0SiṡSi+1), between neighbor coppers at 4.49 Å along chains connected by non-covalent and H-bonds. We also observe a narrow specific heat peak at 0.89 K indicating a phase transition to a 3D magnetically ordered phase. Magnetization curves at fixed T = 2, 4 and 7 K with B0 between 0 and 9 T, and at T between 2 and 300 K with several fixed values of B0 were globally fitted by an intrachain AFM exchange coupling constant 2J0=(-2.27±0.02) cm-1 and g = 2.091±0.005. Interchain interactions J1 between coppers in neighbor chains connected through long chemical paths with total length of 9.51 Å cannot be estimated from magnetization curves. However, observation of the phase transition in the specific heat data allows estimating the range 0.1≤|2J1|≤0.4 cm-1, covering the predictions of various approximations. We analyze the magnitudes of 2J0 and 2J1 in terms of the structure of the corresponding chemical paths. The main contribution in supporting the intrachain interaction is assigned to H-bonds while the interchain interactions are supported by paths containing H-bonds and carboxylate bridges, with the role of the H-bonds being predominant. We compare the obtained intrachain coupling with studies of compounds showing similar behavior and discuss the validity of the approximations allowing to calculate the interchain
Raising and lowering operators of spin-weighted spheroidal harmonics
NASA Astrophysics Data System (ADS)
Shah, Abhay G.; Whiting, Bernard F.
2016-06-01
Differential operators for raising and lowering angular momentum for spherical harmonics are used widely in many branches of physics. Less well known are raising and lowering operators for both spin and the azimuthal component of angular momentum (Goldberg et al. in J Math Phys 8:2155, 1967). In this paper we generalize the spin-raising and lowering operators of spin-weighted spherical harmonics to operators linear-in-γ for spin-weighted spheroidal harmonics, where γ is an additional parameter present in the second order ordinary differential equation governing these harmonics. Constructing these operators has required using all the ℓ -, s- and m-raising and lowering operators (and various combinations of them) for spin-weighted spherical harmonics, which have been calculated and shown explicitly in this paper. Following a well-defined procedure, the operators given could be generalized to higher powers in γ.
Abdalrahman, T; Scheiner, S; Hellmich, C
2015-01-21
It is generally agreed on that trabecular bone permeability, a physiologically important quantity, is governed by the material׳s (vascular or intertrabecular) porosity as well as by the viscosity of the pore-filling fluids. Still, there is less agreement on how these two key factors govern bone permeability. In order to shed more light onto this somewhat open issue, we here develop a random homogenization scheme for upscaling Poiseuille flow in the vascular porosity, up to Darcy-type permeability of the overall porous medium "trabecular bone". The underlying representative volume element of the macroscopic bone material contains two types of phases: a spherical, impermeable extracellular bone matrix phase interacts with interpenetrating cylindrical pore channel phases that are oriented in all different space directions. This type of interaction is modeled by means of a self-consistent homogenization scheme. While the permeability of the bone matrix equals to zero, the permeability of the pore phase is found through expressing the classical Hagen-Poiseuille law for laminar flow in the format of a "micro-Darcy law". The upscaling scheme contains pore size and porosity as geometrical input variables; however, they can be related to each other, based on well-known relations between porosity and specific bone surface. As two key results, validated through comprehensive experimental data, it appears (i) that the famous Kozeny-Carman constant (which relates bone permeability to the cube of the porosity, the square of the specific surface, as well as to the bone fluid viscosity) needs to be replaced by an again porosity-dependent rational function, and (ii) that the overall bone permeability is strongly affected by the pore fluid viscosity, which, in case of polarized fluids, is strongly increased due to the presence of electrically charged pore walls. PMID:25452137
NASA Astrophysics Data System (ADS)
Lasič, Samo; Szczepankiewicz, Filip; Eriksson, Stefanie; Nilsson, Markus; Topgaard, Daniel
2014-02-01
Diffusion tensor imaging (DTI) is the method of choice for non-invasive investigations of the structure of human brain white matter. The results are conventionally reported as maps of the fractional anisotropy (FA), which is a parameter related to microstructural features such as axon density, diameter, and myelination. The interpretation of FA in terms of microstructure becomes ambiguous when there is a distribution of axon orientations within the image voxel. In this paper, we propose a procedure for resolving this ambiguity by determining a new parameter, the microscopic fractional anisotropy (µFA), which corresponds to the FA without the confounding influence of orientation dispersion. In addition, we suggest a method for measuring the orientational order parameter (OP) for the anisotropic objects. The experimental protocol is capitalizing on a recently developed diffusion NMR pulse sequence based on magic-angle spinning of the q-vector. Proof-of-principle experiments are carried out on microimaging and clinical MRI equipment using lyotropic liquid crystals and plant tissues as model materials with high µFA and low FA on account of orientation dispersion. We expect the presented method to be especially fruitful in combination with DTI and high angular resolution acquisition protocols for neuroimaging studies of grey and white matter.
Spin ordering between sub-lattices in nasicon Li3Fe2(PO4)3 measured by Mössbauer spectroscopy
NASA Astrophysics Data System (ADS)
Kim, Hee Seung; Kim, Chul Sung
2013-05-01
The chemical stability and conductivity of nasicon-structured α-Li3Fe2(PO4)3 make it a possible candidate for a cathode material in Li-battery. The x-ray diffraction pattern of Li3Fe2(PO4)3 showed the monoclinic structure with space group of P21/n. In the zero-field-cooled (ZFC) curve, the magnetization remained constant while the temperature was increased up to the splitting temperature (TS = 11 K) of two sub-lattices, indicating the antiferromagnetic behavior below TS. Magnetization curves of both ZFC and FC from 4.2 to 295 K showed ferrimagnetic behavior below the Néel temperature (TN = 29.5 K). We observed the change in the slope of the temperature-dependent Hhf curve at TS. These results suggest that the change in the spin ordering in Li3Fe2(PO4)3 is originated from the difference in hyperfine interactions between the localized Fe3+ magnetic ions at each of two sub-lattices. The spectra of Li3Fe2(PO4)3 under applied magnetic field of 5 T exhibit the magnetic phase transition around TS, indicating antiferromagnetic behavior below TS and ferrimagnetic behavior between TS and TN.
Liu, Guang-Hua; You, Wen-Long; Li, Wei; Su, Gang
2015-04-29
Quantum phase transitions (QPTs) and the ground-state phase diagram of the spin-1/2 Heisenberg-Ising alternating chain (HIAC) with uniform Dzyaloshinskii-Moriya (DM) interaction are investigated by a matrix-product-state (MPS) method. By calculating the odd- and even-string order parameters, we recognize two kinds of Haldane phases, i.e. the odd- and even-Haldane phases. Furthermore, doubly degenerate entanglement spectra on odd and even bonds are observed in odd- and even-Haldane phases, respectively. A rich phase diagram including four different phases, i.e. an antiferromagnetic (AF), AF stripe, odd- and even-Haldane phases, is obtained. These phases are found to be separated by continuous QPTs: the topological QPT between the odd- and even-Haldane phases is verified to be continuous and corresponds to conformal field theory with central charge c = 1; while the rest of the phase transitions in the phase diagram are found to be c = 1/2. We also revisit, with our MPS method, the exactly solvable case of HIAC model with DM interactions only on odd bonds and find that the even-Haldane phase disappears, but the other three phases, i.e. the AF, AF stripe and odd-Haldane phases, still remain in the phase diagram. We exhibit the evolution of the even-Haldane phase by tuning the DM interactions on the even bonds gradually. PMID:25817273
NASA Astrophysics Data System (ADS)
Ivanov, S. A.; Beran, P.; Bazuev, G. V.; Ericsson, T.; Tellgren, R.; Anil Kumar, P.; Nordblad, P.; Mathieu, R.
2015-03-01
Stoichiometric polycrystalline samples of L n F e2 /3M o1 /3O3(L n =Nd ,Pr ,Ce ,La ) have been prepared by solid-state reaction and studied by means of x-ray and neutron powder diffraction as well as Mössbauer spectroscopy and magnetic measurements. All samples were found to be of single phase and to have Pnma symmetry with valence state +3 of Fe and Mo. It is demonstrated that the B-site cations of L n F e2 /3M o1 /3O3 in accord with L n Fe O3 order in a G-type antiferromagnetic structure with the magnetic moments aligned along the b axis. However, with significantly lower Néel temperatures than their L n Fe O3 parent compounds. The Fe-O-Fe bond lengths and bond angles and thus the magnitude of the antiferromagnetic superexchange interaction are found to systematically change with the ionic radius of Ln such that TN increases with increasing radius. Only the CeF e2 /3M o1 /3O3 compound experiences a low temperature spin reorientation from alignment along the b axis to the a axis.
NASA Astrophysics Data System (ADS)
Liu, Guang-Hua; You, Wen-Long; Li, Wei; Su, Gang
2015-04-01
Quantum phase transitions (QPTs) and the ground-state phase diagram of the spin-1/2 Heisenberg-Ising alternating chain (HIAC) with uniform Dzyaloshinskii-Moriya (DM) interaction are investigated by a matrix-product-state (MPS) method. By calculating the odd- and even-string order parameters, we recognize two kinds of Haldane phases, i.e. the odd- and even-Haldane phases. Furthermore, doubly degenerate entanglement spectra on odd and even bonds are observed in odd- and even-Haldane phases, respectively. A rich phase diagram including four different phases, i.e. an antiferromagnetic (AF), AF stripe, odd- and even-Haldane phases, is obtained. These phases are found to be separated by continuous QPTs: the topological QPT between the odd- and even-Haldane phases is verified to be continuous and corresponds to conformal field theory with central charge c = 1 while the rest of the phase transitions in the phase diagram are found to be c = 1/2. We also revisit, with our MPS method, the exactly solvable case of HIAC model with DM interactions only on odd bonds and find that the even-Haldane phase disappears, but the other three phases, i.e. the AF, AF stripe and odd-Haldane phases, still remain in the phase diagram. We exhibit the evolution of the even-Haldane phase by tuning the DM interactions on the even bonds gradually.
Spin waves in a persistent spin-current Fermi liquid
Feldmann, J. D.; Bedell, K. S.
2010-06-15
We report two theoretical results for transverse spin waves, which arise in a system with a persistent spin current. Using Fermi liquid theory, we introduce a spin current in the ground state of a polarized or unpolarized Fermi liquid, and we derive the resultant spin waves using the Landau kinetic equation. The resulting spin waves have a q{sup 1} and q{sup 1/2} dispersion to leading order for the polarized and unpolarized systems, respectively.
Tanasa, Radu; Stancu, Alexandru; Enachescu, Cristian; Laisney, Jérôme; Boillot, Marie-Laure
2014-01-20
We discuss the influence of the embedding matrix on the thermal hysteretic behavior of spin transition microparticles of Fe(phen){sub 2}(NCS){sub 2} by using a series of experimental first order reversal curves (FORCs). The shape of FORCs supports the hypothesis considering additional interactions between the spin-transition microparticles and the embedding matrix, which compares to a negative pressure on the particles. A mean-field approach based on negative variable external pressures, together with a cut off/switch on of particles-matrix interactions accounts for the experimental features.
NASA Astrophysics Data System (ADS)
Becker, Katie
Government regulation of food products, food processing, and food preparation is imperative in bringing an unadulterated, nonmisleading, and safe food product to market and is relevant to all areas of food science, including engineering, processing, chemistry, and microbiology. The liability associated with providing consumers with an adulterated or substandard product cannot only tarnish a company's name and reputation, but also impose substantial financial repercussions on the company and those individuals who play an active role in the violation. In order for a company to fully comply with the relevant food laws (both federal and state), an intimate knowledge of food science is required. Individuals knowledgeable in food science play an integral role not only in implementing and counseling food companies/processors to ensure compliance with government regulations, but these individuals are also necessary to the state and federal governments that make and enforce the relevant laws and regulators.
Spin-orbital short-range order in the honeycomb-based quantum magnet Ba3CuSb2O9
NASA Astrophysics Data System (ADS)
Nakatsuji, Satoru
2013-03-01
The realization of quantum correlated matter beyond one dimension has been vigorously pursued in geometrically frustrated spin systems for decades. In frustrated magnetic materials, however, symmetry breaking of orbital and chemical origin is usually found to induce semi-classical spin freezing. In this talk, I present a contrast case where spins and possibly orbitals remain in a liquid state down to low temperature even in a highly disordered structure of 6H-perovskite Ba3CuSb2O9. Our comprehensive experimental analysis indicates that the geometrical frustration of Wannier's Ising antiferromagnet on a triangular lattice can be exploited to build a nano-structured bipartite honeycomb lattice from electric dipolar spin-1/2 molecules. Despite a strong local Jahn-Teller distortion about the Cu2+ ion, the resulting spin-orbital random bond lattice not only retains hexagonal symmetry averaged over time and space, but it supports a gapless excitation spectrum without spin freezing down to ultralow temperatures. This is the work based on the collaboration with K. Kuga, K. Kimura, R. Satake, N. Katayama, E. Nishibori, H. Sawa, R. Ishii, M. Hagiwara, F. Bridges, T. U. Ito, W. Higemoto, Y. Karaki, M. Halim, A. A. Nugroho, J. A. Rodriguez-Rivera, M. A. Green, C. Broholm. This work is partially supported by Grant-in-Aid for Scientific Research (No. 20340089,21684019) from JSPS, by Grant-in-Aid for Scientific Research on Priority Areas (No. 1951010,19052003) from MEXT, Japan.
Shiomi, Y; Saitoh, E
2014-12-31
We have demonstrated spin pumping from a paramagnetic state of an insulator La2NiMnO6 into a Pt film. Single-crystalline films of La2NiMnO6 which exhibit a ferromagnetic order at TC≈270 K were grown by pulsed laser deposition. The inverse spin Hall voltage induced by spin-current injection has been observed in the Pt layer not only in the ferromagnetic phase of La2NiMnO6, but also in a wide temperature range above TC. The efficient spin pumping in the paramagnetic phase is ascribable to ferromagnetic correlation, not to ferromagnetic order. PMID:25615367
NASA Astrophysics Data System (ADS)
Kawame, Yu; Akushichi, Taiju; Takamura, Yota; Shuto, Yusuke; Sugahara, Satoshi
2015-05-01
We successfully fabricate a (100)-orientated B2-type-Co2FeSi0.5Al0.5 (CFSA)/MgO/Si(100) tunnel contact that is promising for an efficient spin injector for Si channels. The MgO barrier is formed by radical oxidation of an Mg thin film deposited on a Si(100) surface at room temperature and successive radical oxygen annealing at 400 °C. The CFSA electrode is grown on the MgO barrier at 400 °C by ultrahigh-vacuum molecular beam deposition, and it exhibits a (100)-orientated columnar polycrystalline structure with a high degree (63%) of B2-order. The MgO barrier near the interface of the CFSA/MgO junction is crystallized with the (100) orientation, i.e., the spin filter effect due to the MgO barrier could be expected for this junction. A three-terminal Si-channel spin-accumulation device with a CFSA/MgO/Si(100) spin injector is fabricated, and the Hanle effect of accumulated spin polarized electrons injected from this contact to the Si channel is observed.
Kawame, Yu Akushichi, Taiju; Shuto, Yusuke; Sugahara, Satoshi; Takamura, Yota
2015-05-07
We successfully fabricate a (100)-orientated B2-type-Co{sub 2}FeSi{sub 0.5}Al{sub 0.5} (CFSA)/MgO/Si(100) tunnel contact that is promising for an efficient spin injector for Si channels. The MgO barrier is formed by radical oxidation of an Mg thin film deposited on a Si(100) surface at room temperature and successive radical oxygen annealing at 400 °C. The CFSA electrode is grown on the MgO barrier at 400 °C by ultrahigh-vacuum molecular beam deposition, and it exhibits a (100)-orientated columnar polycrystalline structure with a high degree (63%) of B2-order. The MgO barrier near the interface of the CFSA/MgO junction is crystallized with the (100) orientation, i.e., the spin filter effect due to the MgO barrier could be expected for this junction. A three-terminal Si-channel spin-accumulation device with a CFSA/MgO/Si(100) spin injector is fabricated, and the Hanle effect of accumulated spin polarized electrons injected from this contact to the Si channel is observed.
Spin Circuit Representation for Spin Pumping Phenomena
NASA Astrophysics Data System (ADS)
Roy, Kuntal; Datta, Supriyo
2015-03-01
There has been enormous progress in the field of spintronics and nanomagnetics in recent years with the discovery of many new materials and phenomena and it remains a formidable challenge to integrate these phenomena into functional devices and evaluate their potential. To facilitate this process a modular approach has been proposed whereby different phenomena are represented by spin circuit components. Unlike ordinary circuit components, these spin circuit components are characterized by 4-component voltages and currents (one for charge and three for spin). In this talk we will (1) present a spin circuit representation for spin pumping phenomena, (2) combine it with a spin circuit representation for the spin Hall effect to show that it reproduces established results obtained earlier by other means, and finally (3) use it to propose a possible method for enhancing the spin pumping efficiency by an order of magnitude through the addition of a spin sink layer. This work was supported by FAME, one of six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA.
Spin-orbit torques and anisotropic magnetization damping in skyrmion crystals
NASA Astrophysics Data System (ADS)
Hals, Kjetil M. D.; Brataas, Arne
2014-02-01
The length scale of the magnetization gradients in chiral magnets is determined by the relativistic Dzyaloshinskii-Moriya interaction. Thus, even conventional spin-transfer torques are controlled by the relativistic spin-orbit coupling in these systems, and additional relativistic corrections to the current-induced torques and magnetization damping become important for a complete understanding of the current-driven magnetization dynamics. We theoretically study the effects of reactive and dissipative homogeneous spin-orbit torques and anisotropic damping on the current-driven skyrmion dynamics in cubic chiral magnets. Our results demonstrate that spin-orbit torques play a significant role in the current-induced skyrmion velocity. The dissipative spin-orbit torque generates a relativistic Magnus force on the skyrmions, whereas the reactive spin-orbit torque yields a correction to both the drift velocity along the current direction and the transverse velocity associated with the Magnus force. The spin-orbit torque corrections to the velocity scale linearly with the skyrmion size, which is inversely proportional to the spin-orbit coupling. Consequently, the reactive spin-orbit torque correction can be the same order of magnitude as the nonrelativistic contribution. More importantly, the dissipative spin-orbit torque can be the dominant force that causes a deflected motion of the skyrmions if the torque exhibits a linear or quadratic relationship with the spin-orbit coupling. In addition, we demonstrate that the skyrmion velocity is determined by anisotropic magnetization damping parameters governed by the skyrmion size.
NASA Astrophysics Data System (ADS)
Franke, Deanna; Maxwell, Robert; Lathrop, David; Banks, Kesha; Eckert, Hellmut
1992-10-01
The structure of glasses in the system CdGeAs2-xPx is discussed on the basis of complementary solid-state NMR experiments, including 31P and 113Cd magic-angle spinning (MAS) and spin-echo techniques, as well as 31-113Cd spin-echo double resonance (SEDOR) NMR. Computer simulations of atomic distribution models and experimental studies on crystalline model systems are used to quantify the results. The analysis reveals striking differences in the short-range order between the glassy and the stoichiometrically analogous crystalline materials. The structure of glasses in the system CdGeAs2-xPx is characterized by the presence of a substantial fraction of homopolar pnictogen-pnictogen bonds and by a distribution of cadmium relative to phosphorus that is close to random. These results lend credence to the bond-switching model invoked for the structural description of amorphous tetrahedral semiconductors.
NASA Astrophysics Data System (ADS)
Geng, Rugang; Roy, Anandi; Subedi, Ram; Locklin, Jason; Nguyen, Tho; Zhao, Wenbo; Li, Xiaoguang
Charge transport in amorphous organic semiconductors is governed by carriers hopping between localized states with small spin diffusion length. Furthermore, the spin interfacial resistance of organic spin valves (OSVs) is poorly controlled resulting in controversial reports of the magnetoresistance response. Here, we used surface initiated Kumada transfer polycondensation to covalently graft π-conjugated poly(3-methylthiophene) brushes from the La0.67Sr0.33MnO3 (LSMO) bottom electrode. The covalent attachment along with the brush morphology allows for more control over the LSMO/brush interfacial resistance and large spacer mobility. Remarkably, with 15 nm brush spacer layer, we observed an optimum magnetoresistance (MR) effect of 70% at cryogenic temperatures and a MR of 2.7% at 280K. The temperature dependence of the MR is nearly an order of magnitude weaker than that found in control OSVs made from spin-coated poly(3-hexylthiophene). Using a variety of different brush layer thicknesses, the thickness dependent MR at 20K was investigated. A spin diffusion length of 20 nm at 5 mV junction voltage rapidly increases to 55 nm at -280 mV. We acknowledge NSF (CHE 1412714 and DMR 0953112) (J.L.), the UGA start-up funds and Faculty Research Grant (T.N.), NSFC and NBRPC (2012CB922003 and 2015CB921201, X.G.L.) for funding this work.
Unstable spin-ice order in the stuffed metallic pyrochlore Pr_{2+x}Ir_{2-x}O_{7-δ}
MacLaughlin, D. E.; Bernal, O. O.; Shu, Lei; Ishikawa, Jun; Matsumoto, Yosuke; Wen, Jia -Jia; Mourigal, Martin P.; Stock, C.; Ehlers, Georg; Broholm, C. L.; Machida, Yo; Kimura, Kenta; Nakatsuji, Satoru; Shimura, Yasuyuki; Sakakibara, Toshiro
2015-08-24
Specific heat, elastic neutron scattering, and muon spin rotation experiments have been carried out on a well-characterized sample of “stuffed” (Pr-rich) Pr_{2+x}Ir_{2-x}O_{7-δ}. Elastic neutron scattering shows the onset of long-range spin-ice “2-in/2-out” magnetic order at 0.93 kelvin, with an ordered moment of 1.7(1) Bohr magnetons per Pr ion at low temperatures. Approximate lower bounds on the correlation length and correlation time in the ordered state are 170 angstroms and 0.7 nanosecond, respectively. Muon spin rotation experiments yield an upper bound 2.6(7) milliteslas on the local field B^{4f}_{loc} at the muon site, which is nearly two orders of magnitude smaller than the expected dipolar field for long-range spin-ice ordering of 1.7-Bohr magneton moments (120–270 milliteslas, depending on the muon site). This shortfall is due in part to splitting of the non-Kramers crystal-field ground-state doublets of near-neighbor Pr^{3+} ions by the positive-muon-induced lattice distortion. For this to be the only effect, however, ~160 Pr moments out to a distance of ~14 angstroms must be suppressed. An alternative scenario—one consistent with the observed reduced nuclear hyperfine Schottky anomaly in the specific heat—invokes slow correlated Pr-moment fluctuations in the ordered state that average B^{4f}_{loc} on the μSR time scale (~10^{-7} second), but are static on the time scale of the elastic neutron scattering experiments (~10^{-9} second). In this picture, the dynamic muon relaxation suggests a Pr^{3+} 4f correlation time of a few nanoseconds, which should be observable in a neutron spin echo experiment.
Spin-dependent shot noise in semiconductor and graphene nanostructures
NASA Astrophysics Data System (ADS)
Dragomirova, Ralitsa L.
Shot noise is the name given to the time-dependent non-equilibrium current (or voltage) fluctuations which persist down to zero temperature and are fundamentally related to the discrete nature of the electron charge. Over the past two decades it has become a major tool for gathering information about microscopic mechanisms of transport and correlations between charges which cannot be extracted from traditional conductance measurements. Recently a handful of theoretical and experimental studies have suggested that shot noise in systems with spin-dependent interactions provides a sensitive probe to differentiate between scattering from magnetic impurities, spin-flip scattering, and continuous spin precession effects on semiclassical or quantum transport of injected spin-polarized currents. This is due to the fact that any spin flip converts spin-↑ subsystem particle into a spin-↓ subsystem particle, where the two subsystems differ when spin degeneracy is lifted. Thus, the nonconservation of the number of particles in each subsystem generates additional source of current fluctuations. Here we generalize the scattering theory of quantum shot noise to include the full spin-density matrix of electrons. This formalism yields the spin-resolved shot noise power applicable for a generic spintronic device where partially polarized charge current or even pure spin current is injected from a spin-filtering or ferromagnetic electrode into a quantum-coherent nanostructure governed by arbitrary spin-dependent interactions. The developed formalism [2, 5] is applied in Chapter 5 to diffusive multichannel quantum wires with the Rashba spin-orbit (SO) coupling sandwiched between ferromagnetic source and ferromagnetic or normal drain electrodes. The crucial role played by the SO interactions in all-electrical control of spin in semiconductor nanostructures has ignited recent studies of their signatures on the shot noise. We investigate what is the effect of the Rahsba SO coupling
Squeezed spin states: Squeezing the spin uncertainty relations
NASA Technical Reports Server (NTRS)
Kitagawa, Masahiro; Ueda, Masahito
1993-01-01
The notion of squeezing in spin systems is clarified, and the principle for spin squeezing is shown. Two twisting schemes are proposed as building blocks for spin squeezing and are shown to reduce the standard quantum noise, s/2, of the coherent S-spin state down to the order of S(sup 1/3) and 1/2. Applications to partition noise suppression are briefly discussed.
NASA Astrophysics Data System (ADS)
Woods, Justin; Bhat, Vinayak; Farmer, Barry; Sklenar, Joseph; Teipel, Eric; Ketterson, John; Hastings, J. Todd; de Long, Lance
2015-03-01
Artificial spin ice (ASI) systems are composed of nanoscale ferromagnetic segments whose shape anisotropy dictates they behave as mesoscopic Ising spins. Most ASI have segments patterned on periodic lattices and a single vertex topology. We have continuously distorted 2D honeycomb and square lattices such that the pattern vertex spacings follow a Fibonacci chain sequence along primitive lattice directions. The Fibonacci distortion is related to the aperiodic translational symmetry of 2D artificial quasicrystals1 that cannot be viewed as continuous distortions of periodic lattices due to their forbidden (e.g., fivefold) rotational symmetries. In contrast, Fibonacci distortions of 2D periodic lattices can be ``turned on'' by control of the ratio of two lattice parameters d1 and d2. Distortions alter film segments such that pattern vertices are no longer equivalent and traditional spin ice rules are no longer strictly valid. We have performed OOMMF simulations of magnetization reversal for samples having different levels of distortion, and found the magnetic reversal to be dramatically slowed by small distortions (d1/d2 ~ 1). Research at Kentucky is supported by U.S. DoE Grant DE-FG02-97ER45653 and NSF Grant EPS-0814194.
Ewings, R. A.; Perring, T. G.; Sikora, O.; Abernathy, D. L.; Tomioka, Y.; Tokura, Y.
2016-07-06
We have used time-of-flight inelastic neutron scattering to measure the spin wave spectrum of the canonical half-doped manganite Pr0.5Ca0.5MnO3 in its magnetic and orbitally ordered phase. Comparison of the data, which cover multiple Brillouin zones and the entire energy range of the excitations, with several different models shows that only the CE-type ordered state provides an adequate description of the magnetic ground state, provided interactions beyond nearest neighbor are included. We are able to rule out a ground state in which there exist pairs of dimerized spins which interact only with their nearest neighbors. The Zener polaron ground state, whichmore » comprises strongly bound magnetic dimers, can be ruled out on the basis of gross features of the observed spin wave spectrum. A model with weaker dimerization reproduces the observed dispersion but can be ruled out on the basis of subtle discrepancies between the calculated and observed structure factors at certain positions in reciprocal space. Adding further neighbor interactions results in almost no dimerization, i.e. interpolating back to the CE model. These results are consistent with theoretical analysis of the degenerate double exchange model for half-doping.« less
NASA Astrophysics Data System (ADS)
García-Muñoz, José Luis; Padilla-Pantoja, Jessica; Torrelles, Xavier; Blasco, Javier; Herrero-Martín, Javier; Bozzo, Bernat; Rodríguez-Velamazán, José A.
2016-07-01
In half-doped P r0.50A0.50Co O3 metallic perovskites, the spin-lattice coupling brings about distinct magnetostructural transitions for A =Ca and A =Sr at temperatures close to ˜100 K. However, the ground magnetic properties of P r0.50S r0.50Co O3 (PSCO) strongly differ from P r0.50C a0.50Co O3 ones, where a partial P r3 + to P r4 + valence shift and Co spin transition makes the system insulating below the transition. This paper investigates and describes the relationship between the I m m a →I 4 /m c m symmetry change [Padilla-Pantoja, García-Muñoz, Bozzo, Jirák, and Herrero-Martín, Inorg. Chem. 53, 12297 (2014)] and the original magnetic behavior of PSCO versus temperature and external magnetic fields. The FM1 and FM2 ferromagnetic phases, above and below the magnetostructural transition (TS 1˜120 K ) have been investigated. The FM2 phase of PSCO is composed of [100] FM domains, with magnetic symmetry I m'm'a (mx≠0 , mz=0 ). The magnetic space group of the FM1 phase is F m'm'm (with mx=my ). Neutron data analyses in combination with magnetometry and earlier reports results agrees with a reorientation of the magnetization axis by 45∘ within the a b plane across the transition, in which the system retains its metallic character. The presence below TS 1 of conjugated magnetic domains, both of F m'm'm symmetry but having perpendicular spin orientations along the diagonals in the x y plane of the tetragonal unit cell, is at the origin of the anomalies observed in the macroscopic magnetization. A relatively small field μ0H [⊥ z ] ≳30 mT is able to reorient the magnetization within the a b plane, whereas a higher field (μ0H [∥z ] ≳1.2 T at 2 K) is necessary to align the Co moments perpendicular to the a b plane. Such a spin reorientation, in which the orbital and spin components of the Co moment rotate joined by 45∘, was not observed previously in analogous cobaltites without praseodymium.
Solvent removal during synthetic and Nephila fiber spinning.
Kojic, Nikola; Kojic, Milos; Gudlavalleti, Sauri; McKinley, Gareth
2004-01-01
The process by which spiders make their mechanically superior fiber involves removal of solvent (water) from a concentrated protein solution while the solution flows through a progressively narrowing spinning canal. Our aim was to determine a possible mechanism of spider water removal by using a computational model. To develop appropriate computational techniques for modeling of solvent removal during fiber spinning, a study was first performed using a synthetic solution. In particular, the effect of solvent removal during elongational flow (also exhibited in the spinning canal of the spider) on fiber mechanical properties was examined. The study establishes a model for solvent removal during dry spinning of synthetic fibers, assuming that internal diffusion governs solvent removal and that convective resistance is small. A variable internal solvent diffusion coefficient, dependent on solvent concentration, is also taken into account in the model. An experimental setup for dry (air) spinning was used to make fibers whose diameter was on the order of those made by spiders (approximately 1 microm). Two fibers of different thickness, corresponding to different spinning conditions, were numerically modeled for solvent removal and then mechanically tested. These tests showed that the thinner fiber, which lost more solvent under elongational flow, had 5-fold better mechanical properties (elastic modulus of 100 MPa and toughness of 15 MJ/m3) than the thicker fiber. Even though the mechanical properties were far from those of dragline spider silk (modulus of 10 GPa and toughness of 150 MJ/m3), the experimental methodology and numerical principles developed for the synthetic case proved to be valuable when establishing a model for the Nephila spinning process. In this model, an assumption of rapid convective water removal at the spinning canal wall was made, with internal diffusion of water through the fiber as the governing process. Then the diffusion coefficient of water
Spin-orbital driven ferroelectricity
NASA Astrophysics Data System (ADS)
Zhu, Shan; Li, You-Quan
2014-10-01
We study the effect of octahedron rotation on the electric polarization with spin-orbit coupling. Employing local coordinates to represent the tilting of the ligands' octahedra, we evaluate the electric polarization in a chain of transition metal ions with non-polar octahedron rotation. We find the orbital ordering produced by the ligands' rotation and the spin order, together, determine the polarization features, manifesting that non-vanishing polarization appears in collinear spin order and the direction of polarization is no more restricted in the plane of spin rotation in cycloidal ordering.
Yan, J.-Q.; Cao, H. B.; McGuire, M. A.; Ren, Y.; Sales, B. C.; Mandrus, D. G.
2013-06-10
The spin and orbital ordering in Dy₁₋xTbxVO₃ (x=0 and 0.2) was studied by measuring x-ray powder diffraction, magnetization, specific heat, and neutron single-crystal diffraction. The results show that G-OO/C-AF and C-OO/G-AF phases coexist in Dy0.8Tb0.20VO3 in the temperature range 2–60 K, and the volume fraction of each phase is temperature and field dependent. The ordering of Dy moments at T* = 12 K induces a transition from G-OO/C-AF to a C-OO/G-AF phase. Magnetic fields suppress the long-range order of Dy moments and thus the C-OO/G-AF phase below T*. The polarized moments induced at the Dy sublattice by external magnetic fieldsmore » couple to the V 3d moments, and this coupling favors the G-OO/C-AF state. Also discussed is the effect of the Dy-V magnetic interaction and local structure distortion on the spin and orbital ordering in Dy₁₋xTbxVO₃.« less
Yan, J.-Q.; Cao, H. B.; McGuire, M. A.; Ren, Y.; Sales, B. C.; Mandrus, D. G.
2013-06-10
The spin and orbital ordering in Dy₁₋_{x}Tb_{x}VO₃ (x=0 and 0.2) was studied by measuring x-ray powder diffraction, magnetization, specific heat, and neutron single-crystal diffraction. The results show that G-OO/C-AF and C-OO/G-AF phases coexist in Dy_{0.8}Tb_{0.20}VO_{3} in the temperature range 2–60 K, and the volume fraction of each phase is temperature and field dependent. The ordering of Dy moments at T* = 12 K induces a transition from G-OO/C-AF to a C-OO/G-AF phase. Magnetic fields suppress the long-range order of Dy moments and thus the C-OO/G-AF phase below T*. The polarized moments induced at the Dy sublattice by external magnetic fields couple to the V 3d moments, and this coupling favors the G-OO/C-AF state. Also discussed is the effect of the Dy-V magnetic interaction and local structure distortion on the spin and orbital ordering in Dy₁₋_{x}Tb_{x}VO₃.
Geometrical spin symmetry and spin
Pestov, I. B.
2011-07-15
Unification of General Theory of Relativity and Quantum Mechanics leads to General Quantum Mechanics which includes into itself spindynamics as a theory of spin phenomena. The key concepts of spindynamics are geometrical spin symmetry and the spin field (space of defining representation of spin symmetry). The essence of spin is the bipolar structure of geometrical spin symmetry induced by the gravitational potential. The bipolar structure provides a natural derivation of the equations of spindynamics. Spindynamics involves all phenomena connected with spin and provides new understanding of the strong interaction.
NASA Astrophysics Data System (ADS)
Cahill, David G.
The coupling of spin and heat, i.e., spin caloritronics, gives rise to new physical phenomena in nanoscale spin devices and new ways to manipulate local magnetization. Our work in this field takes advantage of recent advances in the measurement and understanding of heat transport at the nanoscale using ultrafast lasers. We use a picosecond duration pump laser pulses as a source of heat and picosecond duration probe laser pulses to detect changes in temperature, spin accumulation, and spin transfer torque using a combination of time-domain thermoreflectance and time-resolved magneto-optic Kerr effect Our pump-probe optical methods enable us to change the temperature of ferromagnetic layers on a picosecond time-scale and generate enormous heat fluxes on the order of 100 GW m-2 that persist for ~ 30 ps. Thermally-driven ultrafast demagnetization of a perpendicular ferromagnet leads to spin accumulation in a normal metal and spin transfer torque in an in-plane ferromagnet. The data are well described by models of spin generation and transport based on differences and gradients of thermodynamic parameters. The spin-dependent Seebeck effect of a perpendicular ferromagnetic layer converts a heat current into spin current, which in turn can be used to exert a spin transfer torque (STT) on a second ferromagnetic layer with in-plane magnetization. Using a [Co,Ni] multilayer as the source of spin, an energy fluence of ~ 4 J m-2 creates thermal STT sufficient to induce ~ 1 % tilting of the magnetization of a 2 nm-thick CoFeB layer.
Yokoo, T.; Raymond, S.; Zheludev, A.; Maslov, S.; Ressouche, E.; Nakamura, M.; Akimitsu, J.
1998-12-01
Linear-chain nickelates with the composition (Nd{sub x}Y{sub 1{minus}x}){sub 2}BaNiO{sub 5} (x=1, x=0.75, x=0.5, and x=0.25) are studied in a series of neutron-scattering experiments. Powder diffraction is used to determine the temperature dependence of the magnetic structure in all four systems. Single-crystal inelastic neutron scattering is employed to investigate the temperature dependence of the Haldane-gap excitations and low-energy spin waves in the x=1 compound Nd{sub 2}BaNiO{sub 5}. The results of these experiments are discussed in the context of the {open_quotes}Haldane chain in a staggered field{close_quotes} model for R{sub 2}BaNiO{sub 5} systems, and quantitative agreement with theory is obtained. {copyright} {ital 1998} {ital The American Physical Society}
NASA Astrophysics Data System (ADS)
Jun Kwon, Woo; Lee, In Kyu; Hyuk Rhee, Chan; Kim, Chul Sung
2012-04-01
The crystal structures of LiFe1-xMnxPO4 (x = 0.1, 0.3, 0.5) samples have been characterized with x-ray diffraction (XRD) and were determined to be orthorhombic with space group Pnma by Rietveld refinement method. The temperature dependence of the magnetization curves showed abnormal antiferromagnetic behavior as well as a decrease in Néel temperature (TN) with Mn substitution from superconducting quantum interference device (SQUID) measurement. The magnetization decreases until the temperature reaches the spin-reorientation temperature (TS), and then increases with temperature up to TN. The Mössbauer spectra of the LiFe1-xMnxPO4 show that the magnetic hyperfine field (Hhf) and electric quadrupole splitting (ΔEQ) values change with increasing temperature, compared to values at TS, which is caused by the strong electric crystalline field originating from distorted octahedral symmetry. The decrease in TS of LiFe1-xMnxPO4 can be explained by the Mn-concentration-dependent crystal field and spin-orbit coupling in the Fe2 + site.
Hayashi, Toshiki; Xiao, Xunwen; Fujiwara, Hideki; Sugimoto, Toyonari; Nakazumi, Hiroyuki; Noguchi, Satoru; Fujimoto, Tsutomu; Yasuzuka, Syuma; Yoshino, Harukazu; Murata, Keizo; Mori, Takehiko; Aruga-Katori, Hiroko
2006-09-13
The 2:1 salt of a new donor molecule, EDT-DSDTFVSDS with FeBr4- ion, (EDT-DSDTFVSDS)2.FeBr4 showed an essentially metallic behavior despite a small upturn in the electrical resistance below ca. 30 K (electrical conductivities at 290 and 4.2 K are 200 and 170 S cm-1, respectively). The Fe(III) d spins of the FeBr4- ions in this salt were subject to antiferromagnetic ordering at 3.3 K by virtue of a strong pi-d interaction (Jpid) which is comparable to that in a molecular metallic conductor, lambda-(BETS)2.FeCl4, and of a very weak d-d interaction (Jdd). This strong pi-d interaction was evidenced by a large and negative magnetoresistance effect (ca. 20% at 5 T) as well as by the appearance of a large dip in the resistance at the magnetic field (ca. 2.0 T) parallel to the easy axis for the spin-flop transition of the Fe(III) d spins. PMID:16953600
NASA Astrophysics Data System (ADS)
Ruangsri, Uchupol; Vigeland, Sarah J.; Hughes, Scott A.
2016-08-01
A small body orbiting a black hole follows a trajectory that, at leading order, is a geodesic of the black hole spacetime. Much effort has gone into computing "self-force" corrections to this motion, arising from the small body's own contributions to the system's spacetime. Another correction to the motion arises from coupling of the small body's spin to the black hole's spacetime curvature. Spin-curvature coupling drives a precession of the small body, and introduces a "force" (relative to the geodesic) which shifts the small body's worldline. These effects scale with the small body's spin at leading order. In this paper, we show that the equations which govern spin-curvature coupling can be analyzed with a frequency-domain decomposition, at least to leading order in the small body's spin. We show how to compute the frequency of precession along generic orbits, and how to describe the small body's precession and motion in the frequency domain. We illustrate this approach with a number of examples. This approach is likely to be useful for understanding spin coupling effects in the extreme mass ratio limit, and may provide insight into modeling spin effects in the strong field for nonextreme mass ratios.
NASA Astrophysics Data System (ADS)
Dieny, B.; Sousa, R.; Prejbeanu, L.
2007-04-01
Conventional electronics has in the past ignored the spin on the electron, however things began to change in 1988 with the discovery of giant magnetoresistance in metallic thin film stacks which led to the development of a new research area, so called spin-electronics. In the last 10 years, spin-electronics has achieved a number of breakthroughs from the point of view of both basic science and application. Materials research has led to several major discoveries: very large tunnel magnetoresistance effects in tunnel junctions with crystalline barriers due to a new spin-filtering mechanism associated with the spin-dependent symmetry of the electron wave functions new magnetic tunnelling barriers leading to spin-dependent tunnelling barrier heights and acting as spin-filters magnetic semiconductors with increasingly high ordering temperature. New phenomena have been predicted and observed: the possibility of acting on the magnetization of a magnetic nanostructure with a spin-polarized current. This effect, due to a transfer of angular momentum between the spin polarized conduction electrons and the local magnetization, can be viewed as the reciprocal of giant or tunnel magnetoresistance. It can be used to switch the magnetization of a magnetic nanostructure or to generate steady magnetic excitations in the system. the possibility of generating and manipulating spin current without charge current by creating non-equilibrium local accumulation of spin up or spin down electrons. The range of applications of spin electronics materials and phenomena is expanding: the first devices based on giant magnetoresistance were the magnetoresistive read-heads for computer disk drives. These heads, introduced in 1998 with current-in plane spin-valves, have evolved towards low resistance tunnel magnetoresistice heads in 2005. Besides magnetic recording technology, these very sensitive magnetoresistive sensors are finding applications in other areas, in particular in biology. magnetic
NASA Astrophysics Data System (ADS)
Ewings, R. A.; Perring, T. G.; Sikora, O.; Abernathy, D. L.; Tomioka, Y.; Tokura, Y.
2016-07-01
We have used time-of-flight inelastic neutron scattering to measure the spin wave spectrum of the canonical half-doped manganite Pr0.5Ca0.5MnO3 in its magnetic and orbitally ordered phase. The data, which cover multiple Brillouin zones and the entire energy range of the excitations, are compared with several different models that are all consistent with CE-type magnetic order, but arise through different exchange coupling schemes. The Goodenough model, i.e., an ordered state comprising strong nearest-neighbor ferromagnetic interactions along zigzag chains with antiferromagnetic interchain coupling, provides the best description of the data, provided that further neighbor interactions along the chains are included. We are able to rule out a coupling scheme involving formation of strongly bound ferromagnetic dimers, i.e., Zener polarons, on the basis of gross features of the observed spin wave spectrum. A model with weaker dimerization reproduces the observed dispersion but can be ruled out on the basis of discrepancies between the calculated and observed structure factors at certain positions in reciprocal space. Adding further neighbor interactions results in almost no dimerization, i.e., recovery of the Goodenough model. These results are consistent with theoretical analysis of the degenerate double exchange model for half-doping, and provide a recipe for how to interpret future measurements away from half-doping, where degenerate double exchange models predict more complex ground states.
NASA Astrophysics Data System (ADS)
Lan, Jin; Yu, Weichao; Wu, Ruqian; Xiao, Jiang
2015-10-01
A diode, a device allowing unidirectional signal transmission, is a fundamental element of logic structures, and it lies at the heart of modern information systems. The spin wave or magnon, representing a collective quasiparticle excitation of the magnetic order in magnetic materials, is a promising candidate for an information carrier for the next-generation energy-saving technologies. Here, we propose a scalable and reprogrammable pure spin-wave logic hardware architecture using domain walls and surface anisotropy stripes as waveguides on a single magnetic wafer. We demonstrate theoretically the design principle of the simplest logic component, a spin-wave diode, utilizing the chiral bound states in a magnetic domain wall with a Dzyaloshinskii-Moriya interaction, and confirm its performance through micromagnetic simulations. Our findings open a new vista for realizing different types of pure spin-wave logic components and finally achieving an energy-efficient and hardware-reprogrammable spin-wave computer.
Gluonic Spin Contribution to Proton Spin at NLO
Casey, Andrew
2011-05-24
In 1988, when the EMC results showed that the quarks had a much smaller contribution to the spin of the proton than previously thought, the 'Proton Spin Crisis' began. Since then, considerable effort has been directed into discovering the main contributors to proton spin and how much each contributes. One such contributor is the gluonic spin component. QCD NLO evolution equations are combined with boundary conditions obtained from heavy quark decoupling expressions to evolve the equations from infinity to the mass of the charm quark in order to determine the gluonic spin contribution.
NASA Astrophysics Data System (ADS)
Bauer, Gerrit
2009-03-01
The coupling between spin and charge in electronic transport is studied in the field of spintronics. Heat currents are coupled to both charge and spin currents as well [1]. This extension of spintronics to what may be called ``spin caloritronics'' recently enjoys renewed attention [2]. The spin-transfer torque associated with electric currents can excite magnetizations in nanostructures, switching magnetic configuration in spin valves and move domain walls in magnetic wires when exceeding critical values of the order of 10^7Acm-2 [3]. Also heat currents transfer spin angular momentum [4], either intrinsically or via the thermoelectric generation of particle spin currents. We predict that temperature differences of the order of 100 K over typical metallic nanostructures cause effects equivalent to the critical charge current densities. In this talk I will give a brief review of various aspects of spin caloritronics with emphasis on thermal spin transfer torques. This work has been carried out in collaboration with Moosa Hatami, Qinfang Zhang, Paul Kelly, Hans Joakim Skadsem, Arne Brataas and Sadamichi Maekawa. [4pt] [1] M. Johnson and R.H. Silsbee, Phys. Rev. B 35, 4959 (1987).[0pt] [2] International Workshop on Spin Caloritronics, Lorentz Center of Leiden University, 9-13 February 2009, http://www.lorentzcenter.nl/lc/web/2009/323/info.php3?wsid=323[0pt] [3] D. C. Ralph and M. D. Stiles, J. Magn. Magn. Mater. 320, 1190 (2008).[0pt] [4] M. Hatami, G.E.W. Bauer, Q. Zhang, and P.J. Kelly, Phys. Rev. Lett. 99, 066603 (2007).
NASA Astrophysics Data System (ADS)
Champagne, Benoît; Kirtman, Bernard
Static longitudinal polarizabilities (α) and second hyperpolarizabilities (γ) of model H2 chains have been calculated at different ab initio levels to address the performance of the recently proposed spin-component-scaled MP2 (SCS-MP2) method (Grimme, J. Chem Phys 2003, 118, 9095). For both α and γ, the SCS-MP2 method improves over the MP2 results in comparison with reference values evaluated at the CCSD(T) level. Differences from the reference are in the range of 4-6% for α and 1-4% for γ. In the case of γ, the SCS-MP2 scheme improves not only over MP2 but also MP4 and CCSD. Further studies are needed on π-conjugated systems to evaluate the generality of these results.
Spin-Orbit Torques and Anisotropic Magnetization Damping in Skyrmion Crystals
NASA Astrophysics Data System (ADS)
Hals, Kjetil; Brataas, Arne
2014-03-01
We theoretically study the effects of reactive and dissipative homogeneous spin-orbit torques and anisotropic damping on the current-driven skyrmion dynamics in cubic chiral magnets. Our results demonstrate that spin-orbit torques play a significant role in the current-induced skyrmion velocity. The dissipative spin-orbit torque generates a relativistic Magnus force on the skyrmions, whereas the reactive spin-orbit torque yields a correction to both the drift velocity along the current direction and the transverse velocity associated with the Magnus force. The spin-orbit torque corrections to the velocity scale linearly with the skyrmion size, which is inversely proportional to the spin-orbit coupling. Consequently, the reactive spin-orbit torque correction can be the same order of magnitude as the non-relativistic contribution. More importantly, the dissipative spin-orbit torque can be the dominant force that causes a deflected motion of the skyrmions if the torque exhibits a linear or quadratic relationship with the spin-orbit coupling. In addition, we demonstrate that the skyrmion velocity is determined by anisotropic magnetization damping parameters governed by the skyrmion size.
NASA Astrophysics Data System (ADS)
Li, Neng; Mo, Yuxiang; Ching, Wai-Yim
2013-11-01
In this work, we assess a full spectrum of properties (chemical bonding, charge distribution, spin ordering, optical, and elastic properties) of Cr2AC (A = Al, Ge) and their hypothetical nitride counterparts Cr2AN (A = Al, Ge) based on density functional theory calculations. The calculated total energy values indicate that a variety of spin ordering of these four compounds depending on interlayer-interactions between M-A and M-X within the sublattice, which is supported by bonding analysis. MAX phase materials are discovered to possess exotic magnetic properties which indicates that these materials could serve as promising candidates for novel layered magnetic materials for various electronic and spintronic applications. Further analysis of optical properties for two polarization vectors of Cr2AX shows that the reflectivity is high in the visible-ultraviolet region up to ˜15 eV suggesting Cr2AX as a promising candidate for use as a coating material. The elastic coefficients (Cij) and bulk mechanical properties [bulk modulus (K), shear modulus (G), Young's modulus (E), Poisson's ratio (η), and Pugh ratio (G/K)] of these four Cr2AX compounds are also calculated and analyzed, which pave the way to predict or design new MAX phases that are less brittle or tougher by having a lower G/K value or higher η.
Li, Neng; Mo, Yuxiang; Ching, Wai-Yim
2013-11-14
In this work, we assess a full spectrum of properties (chemical bonding, charge distribution, spin ordering, optical, and elastic properties) of Cr{sub 2}AC (A = Al, Ge) and their hypothetical nitride counterparts Cr{sub 2}AN (A = Al, Ge) based on density functional theory calculations. The calculated total energy values indicate that a variety of spin ordering of these four compounds depending on interlayer-interactions between M-A and M-X within the sublattice, which is supported by bonding analysis. MAX phase materials are discovered to possess exotic magnetic properties which indicates that these materials could serve as promising candidates for novel layered magnetic materials for various electronic and spintronic applications. Further analysis of optical properties for two polarization vectors of Cr{sub 2}AX shows that the reflectivity is high in the visible-ultraviolet region up to ∼15 eV suggesting Cr{sub 2}AX as a promising candidate for use as a coating material. The elastic coefficients (C{sub ij}) and bulk mechanical properties [bulk modulus (K), shear modulus (G), Young's modulus (E), Poisson's ratio (η), and Pugh ratio (G/K)] of these four Cr{sub 2}AX compounds are also calculated and analyzed, which pave the way to predict or design new MAX phases that are less brittle or tougher by having a lower G/K value or higher η.
NASA Astrophysics Data System (ADS)
Giri, S. K.; Panda, J.; Nath, T. K.
2012-06-01
The effect of doping of rare earth Pr3+ ion replacing Sm3+ in Sm0.5Sr0.5MnO3 is investigated in details. Measurements of linear and non linear ac magnetic susceptibility, resistivity, magnetoresistance on chemically synthesized (Sm0.5-xPrx)Sr0.5MnO3 shows various interesting features with doping level x=0.15. Here we observe the frequency independent FM-PM transition at higher temperature followed by a frequency dependent re-entered magnetic transition at lower temperature through complex ac susceptibility measurements. We have ascribed our observation to the formation of finite size ferromagnetic clusters which are formed as a consequence of intrinsic phase separation and undergo Spin glass-like freezing below certain temperature in this manganite. The magnetoresistance of the samples also show strong irreversibility with respect to sweeping of the field between highest positive and negative values. All these experimental results have been attributed to phase separation effect and kinetic arrest of electronically phase separated system.
Hatanaka, Takashi; Yoshida, Sumito; Ojino, Mayo; Ishii, Masami
2014-12-01
This research was carried out from the perspective that the damage to the people of Fukushima and others from the Fukushima Daiichi Nuclear Power Station (NPS) accident was an "information disaster." It evaluated the critical problems raised by and actual condition analysis on the process of events in the Fukushima Daiichi NPS disaster and responses of the governments and others, notification of the occurrence of the accident and evacuation order by the national and local governments and the evacuation of residents, and guidance for distribution and intake of stable iodine tablets. The research aimed to provide a basis for the implementation of effective distribution and intake of stable iodine tablets and responses to the "information disaster" in the nuclear power disaster. On March 15 at the time that the most radioactive substances were dispersed, even when the average wind speed at the site area was 1.6 m/s, the radioactive substances had reached the outer boundary of Urgent Protective action planning Zone (UPZ, the region with a radius of 30 km) within about five hours. Because of this, every second counted in the provision of information about the accident and the issuance of evacuation orders. This study evaluated the actual condition of information provision by the national government and others from the perspective of this awareness of the importance of time. On the basis of the results of this kind of consideration, we come to the following recommendations: The Nuclear Emergency Response Guidelines and the system for communication of information to medical providers should be revised. The national government should make preparations for the effective advance distribution and intake of stable iodine tablets. PMID:26557446
Tatara, Gen; Nakabayashi, Noriyuki
2014-05-07
Emergent electromagnetic field which couples to electron's spin in ferromagnetic metals is theoretically studied. Rashba spin-orbit interaction induces spin electromagnetic field which is in the linear order in gradient of magnetization texture. The Rashba-induced effective electric and magnetic fields satisfy in the absence of spin relaxation the Maxwell's equations as in the charge-based electromagnetism. When spin relaxation is taken into account besides spin dynamics, a monopole current emerges generating spin motive force via the Faraday's induction law. The monopole is expected to play an important role in spin-charge conversion and in the integration of spintronics into electronics.
Detection and Control of Individual Nuclear Spins Using a Weakly Coupled Electron Spin
Taminiau, T.H.; Wagenaar, J.J.T.; van der Sar, T.; Jelezko, F.; Dobrovitski, Viatcheslav V.; Hanson, R.
2012-09-28
We experimentally isolate, characterize, and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multipulse sequences on the electron spin that resonantly amplify the interaction with a selected nuclear spin and at the same time dynamically suppress decoherence caused by the rest of the spin bath. We are able to address nuclear spins with interaction strengths that are an order of magnitude smaller than the electron spin dephasing rate. Our results provide a route towards tomography with single-nuclear-spin sensitivity and greatly extend the number of available quantum bits for quantum information processing in diamond.
ERIC Educational Resources Information Center
Morrow, Joyce
Materials for running a student government program at the junior high school level are provided in three general sections. Section 1 is a description of student government operations. Topics covered include student government responsibilities and activities, student council meeting procedures, parliamentary rules, responsibilities of the…
NASA Astrophysics Data System (ADS)
Chai, Jun; Tian, Bo; Zhen, Hui-Ling; Sun, Wen-Rong
2015-11-01
Energy transfer through a (2+1)-dimensional α-helical protein can be described by a (2+1)-dimensional fourth-order nonlinear Schrödinger equation. For such an equation, a Lax pair and the infinitely-many conservation laws are derived. Using an auxiliary function and a bilinear formulation, we get the one-, two-, three- and N-soliton solutions via the Hirota method. The soliton velocity is linearly related to the lattice parameter γ, while the soliton' direction and amplitude do not depend on γ. Interactions between the two solitons are elastic, while those among the three solitons are pairwise elastic. Oblique, head-on and overtaking interactions between the two solitons are displayed. Oblique interaction among the three solitons and interactions among the two parallel solitons and a single one are presented as well.
Zhu, Jian-xin; Dai, Jianhui; Si, Qimiao
2009-01-01
Some of the high {Tc} iron pnictides contain rare-earth elements, raising the question of how the existence and tunability of a d-electron antiferromagnetic order influences the heavy fermion behavior of the f-moments. With CeOFeP and CeOFeAs in mind as prototypes, we derive an extended Anderson lattice model appropriate for these quaternary systems. We show that the Kondo screening of the f-moments are efficiently suppressed by the d-electron ordering. We also argue that, inside the d-electron ordered state (as in CeOFeAs), the f-moments provide a rare realization of a quantum frustrated magnet with competing J{sub 1}-J{sub 2}-J{sub 3} interactions in an effective square lattice. Implications ofr the heavy fermion physics in broader contexts are also discussed.
Jiang, Yu; Huq, Ashfia; Booth, Corwin H.; Ehlers, Georg; Greedan, John E.; Gardner, Jason S.
2011-02-11
To understand the origin of the spin-glass state in molybdate pyrochlores, the structure of Tb{sub 2}Mo{sub 2}O{sub 7} is investigated using two techniques: the long-range lattice structure was measured using neutron powder diffraction (NPD), and local structure information was obtained from the extended x-ray absorption fine structure (EXAFS) technique. While the long-range structure appears generally well ordered, enhanced mean-squared site displacements on the O(1) site and the lack of temperature dependence of the strongly anisotropic displacement parameters for both the Mo and O(1) sites indicate some disorder exists. Likewise, the local structure measurements indicate some Mo-Mo and Tb-O(1) nearest-neighbor disorder exists, similar to that found in the related spin-glass pyrochlore, Y{sub 2}Mo{sub 2}O{sub 7}. Although the freezing temperature in Tb{sub 2}Mo{sub 2}O{sub 7}, 25 K, is slightly higher than in Y{sub 2}Mo{sub 2}O{sub 7}, 22 K, the degree of local pair distance disorder is actually less in Tb{sub 2}Mo{sub 2}O{sub 7}. This apparent contradiction is considered in light of the interactions involved in the freezing process.
NASA Astrophysics Data System (ADS)
Wang, Qi-Min; Gao, Yi-Tian; Su, Chuan-Qi; Mao, Bing-Qing; Gao, Zhe; Yang, Jin-Wei
2015-12-01
In this paper, a higher-order (2 + 1) -dimensional nonlinear Schrödinger-type equation is investigated, which describes the nonlinear spin dynamics of the (2 + 1) -dimensional Heisenberg ferromagnetic spin chain with bilinear and biquadratic interaction. Lax pair and infinite-number conservation laws are constructed, which could prove the existence of the multi-soliton solutions. Via the auxiliary function, bilinear forms and dark-soliton solutions are derived. Properties and interaction patterns for the dark solitons are investigated: (i) Effects on the dark solitons arising from the bilinear interaction, biquadratic interaction and lattice parameter are discussed. (ii) Through the asymptotic analysis, elastic and inelastic interaction between the two solitons is discussed analytically and graphically, respectively. Due to the elastic interaction, amplitudes and velocities of the two dark solitons remain unchanged with the distortion of the interaction area, except for certain phase shifts. However, in virtue of the inelastic interaction, amplitudes of the dark solitons reduce to zero, without the distortion. (iii) Elastic interaction among the three dark solitons is investigated, which implies that the properties of the elastic interaction among the three are similar to that between the two, except for the more complicated distortion. Inelastic-elastic interaction is also investigated, which implies that the interaction between the inelastic region and the dark soliton is elastic. (iv) Linear stability analysis is proposed, which is used to analyze the properties of modulation instability and proves that the dark solitons are modulationally stable.
NASA Astrophysics Data System (ADS)
Kim, Inkoo; Lee, Yoon Sup
2014-10-01
We report the formulation and implementation of KRCASPT2, a two-component multi-configurational second-order perturbation theory based on Kramers restricted complete active space self-consistent field (KRCASSCF) reference function, in the framework of the spin-orbit relativistic effective core potential. The zeroth-order Hamiltonian is defined as the sum of nondiagonal one-electron operators with generalized two-component Fock matrix elements as scalar factors. The Kramers symmetry within the zeroth-order Hamiltonian is maintained via the use of a state-averaged density, allowing a consistent treatment of degenerate states. The explicit expressions are derived for the matrix elements of the zeroth-order Hamiltonian as well as for the perturbation vector. The use of a fully variational reference function and nondiagonal operators in relativistic multi-configurational perturbation theory is reported for the first time. A series of initial calculations are performed on the ionization potential and excitation energies of the atoms of the 6p-block; the results display a significant improvement over those from KRCASSCF, showing a closer agreement with experimental results. Accurate atomic properties of the superheavy elements of the 7p-block are also presented, and the electronic structures of the low-lying excited states are compared with those of their lighter homologues.
Orbital- and spin-order sensitive nonlocal screening in Mn 2p X-ray photoemission of La1‑xSrxMnO3
NASA Astrophysics Data System (ADS)
Hariki, A.; Yamanaka, A.; Uozumi, T.
2016-04-01
The Mn 2p X-ray photoemission spectra (XPS) of LaMnO3 (LMO) and hole-doped La0.7Sr0.3MnO3 (LSMO) are investigated using a dp model simulating Mn 3d and O 2p electrons under the perovskite-type crystal structure. The observed 2p XPS features, especially the low-binding-energy structure (LBES) of the 2p3/2 main line, are reproduced well using an impurity Anderson model optimized from the dp model within the dynamical mean-field approximation. The LBES in both compounds is due to the nonlocal screening (NLS) between the neighboring Mn ions in the final state, but the screening character is quite different: The NLS in LSMO directly reflects the character of the ferromagnetic metal, while that in undoped LMO the C-type orbital order between 3x^2-r2 and 3y^2-r2 orbitals in the ab-plane. We emphasize the directive nature of the NLS in the orbital order system, which can be a sensitive probe to the order pattern.
Spin-induced symmetry breaking in orbitally ordered NiCr2O4 and CuCr2O4
NASA Astrophysics Data System (ADS)
Suchomel, Matthew R.; Shoemaker, Daniel P.; Ribaud, Lynn; Kemei, Moureen C.; Seshadri, Ram
2012-08-01
At room temperature, the normal oxide spinels NiCr2O4 and CuCr2O4 are tetragonally distorted and crystallize in the I41/amd space group due to cooperative Jahn-Teller ordering driven by the orbital degeneracy of tetrahedral Ni2+ (t24) and Cu2+ (t25). Upon cooling, these compounds undergo magnetic ordering transitions; interactions are somewhat frustrated for NiCr2O4 but not for CuCr2O4. We employ variable-temperature high-resolution synchrotron x-ray powder diffraction to establish that at the magnetic ordering temperatures there are further structural changes, which result in both compounds distorting to an orthorhombic structure consistent with the Fddd space group. NiCr2O4 exhibits additional distortion, likely within the same space group, at a yet-lower transition temperature of T=30 K. The tetragonal to orthorhombic structural transition in these compounds appears to primarily involve changes in NiO4 and CuO4 tetrahedra.
Nakajima, Yuya; Seino, Junji; Nakai, Hiromi
2016-05-10
An analytical energy gradient for the spin-dependent general Hartree-Fock method based on the infinite-order Douglas-Kroll-Hess (IODKH) method was developed. To treat realistic systems, the local unitary transformation (LUT) scheme was employed both in energy and energy gradient calculations. The present energy gradient method was numerically assessed to investigate the accuracy in several diatomic molecules containing fifth- and sixth-period elements and to examine the efficiency in one-, two-, and three-dimensional silver clusters. To arrive at a practical calculation, we also determined the geometrical parameters of fac-tris(2-phenylpyridine)iridium and investigated the efficiency. The numerical results confirmed that the present method describes a highly accurate relativistic effect with high efficiency. The present method can be a powerful scheme for determining geometries of large molecules, including heavy-element atoms. PMID:27045757
Spin Hall voltages from a.c. and d.c. spin currents
Wei, Dahai; Obstbaum, Martin; Ribow, Mirko; Back, Christian H.; Woltersdorf, Georg
2014-01-01
In spin electronics, the spin degree of freedom is used to transmit and store information. To this end the ability to create pure spin currents—that is, without net charge transfer—is essential. When the magnetization vector in a ferromagnet–normal metal junction is excited, the spin pumping effect leads to the injection of pure spin currents into the normal metal. The polarization of this spin current is time-dependent and contains a very small d.c. component. Here we show that the large a.c. component of the spin currents can be detected efficiently using the inverse spin Hall effect. The observed a.c.-inverse spin Hall voltages are one order of magnitude larger than the conventional d.c.-inverse spin Hall voltages measured on the same device. Our results demonstrate that ferromagnet–normal metal junctions are efficient sources of pure spin currents in the gigahertz frequency range. PMID:24780927
NASA Astrophysics Data System (ADS)
Taddei, Keith M.
With nearly innumerable applications, superconductivity stands as a holy grail in the research of quantum phenomena. Understanding the mechanism that begets the fabled pairing of electrons which leads to zero resistance is the most significant undertaking in order to bring to fruition all of superconductivity's splendor. Yet the interaction which couples electrons in the most promising family of superconductors known as unconventional superconductors, which show the highest Tc's and largest upper critical fields remains a mystery. Intense study over the past several decades on the cuprate superconductors has allowed for the identification of several candidate mechanisms --- cardinal of which is magnetic fluctuations --- however as of yet the question still remains. Recently, the discovery of the iron-based superconductors has provided another fruitful avenue through which this mechanism can be probed. Excitingly in these materials superconductivity not only arises near a magnetic instability - a situation which is expected to be particularly suited for engendering superconductivity should magnetic fluctuations be the pairing mechanism - but also exhibit the microscopic co-existence of the two presumably adversarial phenomena. In the work presented here the powerful techniques of neutron and x-ray diffraction will be used to study two particularly interesting members of this family: the intercalated iron-selenide CsxFe 2--xSe2 and two members of the iron-arsenide 122 family (BaFe2(As1--xPx)2 and Sr1--xNaxFe2As 2). Though isostructural at high temperatures, these two materials behave remarkably differently and the idiosyncratic manifestations of superconductivity and ordered magnetism in either give clues as to how the latter might stabilize the former. The iron-selenides will be shown to exhibit a complex phase space with phase separation leading to stabilization of magnetism and superconductivity in separate phases. The structure, behavior and complex vacancy
Spin Funneling for Enhanced Spin Injection into Ferromagnets.
Sayed, Shehrin; Diep, Vinh Q; Camsari, Kerem Yunus; Datta, Supriyo
2016-01-01
It is well-established that high spin-orbit coupling (SOC) materials convert a charge current density into a spin current density which can be used to switch a magnet efficiently and there is increasing interest in identifying materials with large spin Hall angle for lower switching current. Using experimentally benchmarked models, we show that composite structures can be designed using existing spin Hall materials such that the effective spin Hall angle is larger by an order of magnitude. The basic idea is to funnel spins from a large area of spin Hall material into a small area of ferromagnet using a normal metal with large spin diffusion length and low resistivity like Cu or Al. We show that this approach is increasingly effective as magnets get smaller. We avoid unwanted charge current shunting by the low resistive NM layer utilizing the newly discovered phenomenon of pure spin conduction in ferromagnetic insulators via magnon diffusion. We provide a spin circuit model for magnon diffusion in FMI that is benchmarked against recent experiments and theory. PMID:27374496
Spin Funneling for Enhanced Spin Injection into Ferromagnets
NASA Astrophysics Data System (ADS)
Sayed, Shehrin; Diep, Vinh Q.; Camsari, Kerem Yunus; Datta, Supriyo
2016-07-01
It is well-established that high spin-orbit coupling (SOC) materials convert a charge current density into a spin current density which can be used to switch a magnet efficiently and there is increasing interest in identifying materials with large spin Hall angle for lower switching current. Using experimentally benchmarked models, we show that composite structures can be designed using existing spin Hall materials such that the effective spin Hall angle is larger by an order of magnitude. The basic idea is to funnel spins from a large area of spin Hall material into a small area of ferromagnet using a normal metal with large spin diffusion length and low resistivity like Cu or Al. We show that this approach is increasingly effective as magnets get smaller. We avoid unwanted charge current shunting by the low resistive NM layer utilizing the newly discovered phenomenon of pure spin conduction in ferromagnetic insulators via magnon diffusion. We provide a spin circuit model for magnon diffusion in FMI that is benchmarked against recent experiments and theory.
All-electric spin transistor using perpendicular spins
NASA Astrophysics Data System (ADS)
Kim, Ji Hoon; Bae, Joohyung; Min, Byoung-Chul; Kim, Hyung-jun; Chang, Joonyeon; Koo, Hyun Cheol
2016-04-01
All-electric spin transistor is demonstrated using perpendicular spins in an InAs quantum well channel. For the injection and detection of perpendicular spins in the quantum well channel, we use Tb20Fe62Co18/Co40Fe40B20 electrodes, where the Tb20Fe62Co18 layer produces the perpendicular magnetization and the Co40Fe40B20 layer enhances the spin polarization. In this spin transistor device, a gate-controlled spin signal as large as 80 mΩ is observed at 10 K without an external magnetic field. In order to confirm the spin injection and relaxation independently, we measure the three-terminal Hanle effect with an in-plane magnetic field, and obtain a spin signal of 1.7 mΩ at 10 K. These results clearly present that the electric field is an efficient way to modulate spin orientation in a strong spin-orbit interaction system.
Spin Funneling for Enhanced Spin Injection into Ferromagnets
Sayed, Shehrin; Diep, Vinh Q.; Camsari, Kerem Yunus; Datta, Supriyo
2016-01-01
It is well-established that high spin-orbit coupling (SOC) materials convert a charge current density into a spin current density which can be used to switch a magnet efficiently and there is increasing interest in identifying materials with large spin Hall angle for lower switching current. Using experimentally benchmarked models, we show that composite structures can be designed using existing spin Hall materials such that the effective spin Hall angle is larger by an order of magnitude. The basic idea is to funnel spins from a large area of spin Hall material into a small area of ferromagnet using a normal metal with large spin diffusion length and low resistivity like Cu or Al. We show that this approach is increasingly effective as magnets get smaller. We avoid unwanted charge current shunting by the low resistive NM layer utilizing the newly discovered phenomenon of pure spin conduction in ferromagnetic insulators via magnon diffusion. We provide a spin circuit model for magnon diffusion in FMI that is benchmarked against recent experiments and theory. PMID:27374496
Spin manipulation in nanoscale superconductors
NASA Astrophysics Data System (ADS)
Beckmann, D.
2016-04-01
The interplay of superconductivity and magnetism in nanoscale structures has attracted considerable attention in recent years due to the exciting new physics created by the competition of these antagonistic ordering phenomena, and the prospect of exploiting this competition for superconducting spintronics devices. While much of the attention is focused on spin-polarized supercurrents created by the triplet proximity effect, the recent discovery of long range quasiparticle spin transport in high-field superconductors has rekindled interest in spin-dependent nonequilibrium properties of superconductors. In this review, the experimental situation on nonequilibrium spin injection into superconductors is discussed, and open questions and possible future directions of the field are outlined.
Spin manipulation in nanoscale superconductors.
Beckmann, D
2016-04-27
The interplay of superconductivity and magnetism in nanoscale structures has attracted considerable attention in recent years due to the exciting new physics created by the competition of these antagonistic ordering phenomena, and the prospect of exploiting this competition for superconducting spintronics devices. While much of the attention is focused on spin-polarized supercurrents created by the triplet proximity effect, the recent discovery of long range quasiparticle spin transport in high-field superconductors has rekindled interest in spin-dependent nonequilibrium properties of superconductors. In this review, the experimental situation on nonequilibrium spin injection into superconductors is discussed, and open questions and possible future directions of the field are outlined. PMID:27001949
ERIC Educational Resources Information Center
Carver, John
2000-01-01
The Policy Governance model's philosophical foundations lie in Rousseau's social contract, Greenleaf's servant-leadership, and modern management theory. Policy Governance stresses primacy of the owner-representative role; full-board authority; superintendents as chief executive officers; authoritative prescription of "ends," bounded freedom for…
ERIC Educational Resources Information Center
Osborne, David T.
1993-01-01
Throughout all levels of American government, a shift is taking place from the rigid, wasteful, centralized bureaucracies of the industrial era to the more flexible, entrepreneurial, decentralized government needed to succeed in today's world. This shift has been brought about by an unprecedented, ongoing fiscal crisis that has created a sudden…
Spin polarization transfer by the radical pair mechanism
Zarea, Mehdi Ratner, Mark A.; Wasielewski, Michael R.
2015-08-07
In a three-site representation, we study a spin polarization transfer from radical pair spins to a nearby electron or nuclear spin. The quantum dynamics of the radical pair spins is governed by a constant exchange interaction between the radical pair spins which have different Zeeman frequencies. Radical pair spins can recombine to the singlet ground state or to lower energy triplet states. It is then shown that the coherent dynamics of the radical pair induces spin polarization on the nearby third spin in the presence of a magnetic field. The spin polarization transfer depends on the difference between Zeeman frequencies, the singlet and triplet recombination rates, and on the exchange and dipole-dipole interactions between the different spins. In particular, the sign of the polarization depends on the exchange coupling between radical pair spins and also on the difference between singlet and triplet recombination rate constants.
Spin-Related Transport Affected by Competition Between Spin-Orbit Interaction and Zeeman Effect
NASA Astrophysics Data System (ADS)
Nitta, Junsaku
The spin dynamics in solid state systems is governed by the competition between spin-orbit interaction (SOI) and the Zeeman effect. The SOI couples orbital motion of electron spins with an electric field. The Zeeman effect lifts the spin degeneracy in a magnetic field. In InGaAs-based 2DEGs, it is known that the Rashba SOI energy ESOI can be controlled by an electric field applied on the gate electrode.1 In the presence of SOI, weak localization (WL) due to time reversal symmetric interference changes to weak anti-localization (WAL). We have found crossover from WL to WAL by applying the gate voltage in InGaAs 2DEGs. Applying an in-plane magnetic field to the 2DEG does not affect the orbital motion of the electrons, but only modifies the Zeeman spin splitting energy EZ. This allows tuning the ratio between ESOI and EZ very accurately. We have studied how the interplay between SOI and Zeeman coupling affects the electron transport and the spin dynamics in InGaAs-based 2DEGs. From the quantitative analysis of the magnetoconductance, measured in the presence of an in-plane magnetic field, we conclude that this interplay results in a spin-induced breaking of time reversal symmetry (TRS) and in an enhancement of the spin relaxation time. Both effects are due to a partial alignment of the electron spin along the applied magnetic field, and are found to be in excellent agreement with recent theoretical predictions.2 We find that the electron dephasing time saturates when EZ becomes comparable to ESOI. Moreover, we show that the spin-induced electron dephasing time is a universal function of the ratio EZ/ESOI within the experimental accuracy, i.e. it is independent of any details of the quantum well.3 This universal behavior is explained by the recent theory.4 The suppression of WAL is observed by applying in-plane magnetic field because of the enhancement of the spin relaxation time, and this suppression also appears in narrow InGaAs wires since the effective magnetic
Effects of Dephasing on Spin Lifetime in Ballistic Spin-Orbit Materials
NASA Astrophysics Data System (ADS)
Cummings, Aron W.; Roche, Stephan
2016-02-01
We theoretically investigate spin dynamics in spin-orbit-coupled materials. In the ballistic limit, the spin lifetime is dictated by dephasing that arises from energy broadening plus a nonuniform spin precession. For the case of clean graphene, we find a strong anisotropy with spin lifetimes that can be short even for modest energy scales, on the order of a few ns. These results offer deeper insight into the nature of spin dynamics in graphene, and are also applicable to the investigation of other systems where spin-orbit coupling plays an important role.
Biswas, Ayan K; Atulasimha, Jayasimha; Bandyopadhyay, Supriyo
2015-07-17
In artificial neural networks, neurons are usually implemented with highly dissipative CMOS-based operational amplifiers. A more energy-efficient implementation is a 'spin-neuron' realized with a magneto-tunneling junction (MTJ) that is switched with a spin-polarized current (representing weighted sum of input currents) that either delivers a spin transfer torque or induces domain wall motion in the soft layer of the MTJ to mimic neuron firing. Here, we propose and analyze a different type of spin-neuron in which the soft layer of the MTJ is switched with mechanical strain generated by a voltage (representing weighted sum of input voltages) and term it straintronic spin-neuron. It dissipates orders of magnitude less energy in threshold operations than the traditional current-driven spin neuron at 0 K temperature and may even be faster. We have also studied the room-temperature firing behaviors of both types of spin neurons and find that thermal noise degrades the performance of both types, but the current-driven type is degraded much more than the straintronic type if both are optimized for maximum energy-efficiency. On the other hand, if both are designed to have the same level of thermal degradation, then the current-driven version will dissipate orders of magnitude more energy than the straintronic version. Thus, the straintronic spin-neuron is superior to current-driven spin neurons. PMID:26112081
NASA Astrophysics Data System (ADS)
Hamp, James; Dutton, Sian; Mourigal, Martin; Mukherjee, Paromita; Paddison, Joseph; Ong, Harapan; Castelnovo, Claudio
Spin ice materials provide a rare instance of emergent gauge symmetry and fractionalisation in three dimensions: the effective degrees of freedom of the system are emergent magnetic monopoles, and the extensively many `ice rule' ground states are those devoid of monopole excitations. Two-dimensional (kagome) analogues of spin ice have also been shown to display a similarly rich behaviour. In kagome ice however the ground-state `ice rule' condition implies the presence everywhere of magnetic charges. As temperature is lowered, an Ising transition occurs to a charge-ordered state, which can be mapped to a dimer covering of the dual honeycomb lattice. A second transition, of Kosterlitz-Thouless or three-state Potts type, occurs to a spin-ordered state at yet lower temperatures, due to small residual energy differences between charge-ordered states. Inspired by recent experimental capabilities in growing spin ice samples with selective (layered) substitution of non-magnetic ions, in this work we investigate the fate of the two ordering transitions when individual kagome layers are brought together to form a three-dimensional pyrochlore structure coupled by long range dipolar interactions. We also consider the response to substitutional disorder and applied magnetic fields.
Loos, Gregory P
2003-01-01
Globalization's profound influence on social and political institutions need not be negative. Critics of globalization have often referred to the "Impossible Trinity" because decision-making must 1. respect national sovereignty, 2. develop and implement firm regulation, and 3. allow capital markets to be as free as possible. To many, such goals are mutually exclusive because history conditions us to view policy-making and governance in traditional molds. Thus, transnational governance merely appears impossible because current forms of governance were not designed to provide it. The world needs new tools for governing, and its citizens must seize the opportunity to help develop them. The rise of a global society requires a greater level of generality and inclusion than is found in most policy bodies today. Politicians need to re-examine key assumptions about government. States must develop ways to discharge their regulatory responsibilities across borders and collaborate with neighboring jurisdictions, multilateral bodies, and business. Concepts such as multilateralism and tripartism show great promise. Governments must engage civil society in the spirit of shared responsibility and democratic decision-making. Such changes will result in a renewal of the state's purpose and better use of international resources and expertise in governance. PMID:17208717
NASA Astrophysics Data System (ADS)
Yang, Jin-Wei; Gao, Yi-Tian; Wang, Qi-Min; Su, Chuan-Qi; Feng, Yu-Jie; Yu, Xin
2016-01-01
In this paper, a fourth-order variable-coefficient nonlinear Schrödinger equation is studied, which might describe a one-dimensional continuum anisotropic Heisenberg ferromagnetic spin chain with the octuple-dipole interaction or an alpha helical protein with higher-order excitations and interactions under continuum approximation. With the aid of auxiliary function, we derive the bilinear forms and corresponding constraints on the variable coefficients. Via the symbolic computation, we obtain the Lax pair, infinitely many conservation laws, one-, two- and three-soliton solutions. We discuss the influence of the variable coefficients on the solitons. With different choices of the variable coefficients, we obtain the parabolic, cubic, and periodic solitons, respectively. We analyse the head-on and overtaking interactions between/among the two and three solitons. Interactions between a bound state and a single soliton are displayed with different choices of variable coefficients. We also derive the quasi-periodic formulae for the three cases of the bound states.
Development of an underwater spin facility for combined environment testing
Roach, D.P.; Nusser, M.A.
1991-01-01
In response to a request from the US Government, Sandia National Laboratories has developed an instrumentation system to monitor the conditions along an underwater, rotating drive shaft. It was desired to study the structural integrity and signal acquisition capabilities of the Shaft Instrumentation System (SIS) in an environment which closely simulates the actual deployment conditions. In this manner, the SIS response to ill-defined conditions, such as flow field turbulence or temperature fluctuations, could be determined. An Underwater Spin Facility was developed in order to verify the operation of the instrumentation and telemetric data acquisition system in a combined environment of external pressure, transient axial loads and centrifugal force. The main components of the Underwater Spin Facility are a large, five foot diameter pressure vessel, a dynamically sealed shaft, a drive train assembly and a shaker table interface which is used to apply the axial loads. This paper presents a detailed description of the design of the Underwater Spin Facility. It also discusses the SIS certification test program in order to demonstrate the successful performance of the Underwater Spin Facility. 8 refs., 10 figs.
Chiral spin liquids in arrays of spin chains
NASA Astrophysics Data System (ADS)
Pereira, Rodrigo
The chiral spin liquid proposed by Kalmeyer and Laughlin is a spin analogue of the fractional quantum Hall effect: it has gapped bulk quasiparticles, charge-neutral chiral edge modes and topological order in the ground state. Recently there has been unambiguous numerical evidence that the chiral spin liquid can be stabilized as the ground state of extended Heisenberg models on the kagome lattice. I will talk about an analytical approach to investigate the emergence and the properties of the chiral spin liquid phase in spatially anisotropic 2D lattices. The approach is inspired by ``coupled-wire constructions'' of quantum Hall states: starting from a quasi-1D system, we build towards the 2D limit by coupling Heisenberg chains with three-spin interactions that drive the chiral spin order. Using a renormalization group analysis, we show that the chiral spin liquid is more easily stabilized in the kagome lattice than in the triangular lattice. Moreover, using the conformal field theory that describes single chains, we explicitly construct the operators that create bulk quasiparticles and those that account for the topological degeneracy on the torus. I will also discuss possible extensions of this approach to construct more exotic quantum spin liquids.
NASA Astrophysics Data System (ADS)
Olson Reichhardt, Cynthia; Libal, Andras; Reichhardt, Charles
We examine square and kagome artificial spin ice for colloids confined in arrays of double-well traps. Unlike magnetic artificial spin ices, colloidal and vortex artificial spin ice realizations allow creation of doping sites through double occupation of individual traps. We find that doping square and kagome ice geometries produces opposite effects. For square ice, doping creates local excitations in the ground state configuration that produce a local melting effect as the temperature is raised. In contrast, the kagome ice ground state can absorb the doping charge without generating non-ground-state excitations, while at elevated temperatures the hopping of individual colloids is suppressed near the doping sites. These results indicate that in the square ice, doping adds degeneracy to the ordered ground state and creates local weak spots, while in the kagome ice, which has a highly degenerate ground state, doping locally decreases the degeneracy and creates local hard regions.
Spin transport in hydrogenated graphene
NASA Astrophysics Data System (ADS)
Soriano, David; Van Tuan, Dinh; M-M Dubois, Simon; Gmitra, Martin; Cummings, Aron W.; Kochan, Denis; Ortmann, Frank; Charlier, Jean-Christophe; Fabian, Jaroslav; Roche, Stephan
2015-06-01
In this review we discuss the multifaceted problem of spin transport in hydrogenated graphene from a theoretical perspective. The current experimental findings suggest that hydrogenation can either increase or decrease spin lifetimes, which calls for clarification. We first discuss the spin-orbit coupling induced by local σ -π re-hybridization and {s}{{{p}}3} C-H defect formation together with the formation of a local magnetic moment. First-principles calculations of hydrogenated graphene unravel the strong interplay of spin-orbit and exchange couplings. The concept of magnetic scattering resonances, recently introduced by Kochan et al (2014 Phys. Rev. Lett. 112 116602) is revisited by describing the local magnetism through the self-consistent Hubbard model in the mean field approximation in the dilute limit, while spin relaxation lengths and transport times are computed using an efficient real space order N wavepacket propagation method. Typical spin lifetimes on the order of 1 ns are obtained for 1 ppm of hydrogen impurities (corresponding to a transport time of about 50 ps), and the scaling of spin lifetimes with impurity density is described by the Elliott-Yafet mechanism. This reinforces the statement that local defect-induced magnetism can be at the origin of the substantial spin polarization loss in the clean graphene limit.
Two-step spin flop transition in quantum spin ladders
NASA Astrophysics Data System (ADS)
Sakai, Toru; Okamoto, Kiyomi
2008-03-01
It is well known that the antiferromagnet with easy-axis anisotropies exhibits a field-induced first-order phase transition, the so- called spin flop. In one-dimensional quantum spin systems, instead of it, a second-order phase transition occurs because of large quantum fluctuations[1]. Particularly the S=1 antiferromagnetic chain with the easy-axis single-ion anisotropy was revealed to exhibit two successive field-induced second-order transitions by our previous numerical analysis[2]. However, such transitions have not been obseved yet. Recently a two-step spin flop transition was observed in the spin ladder system IPA-CuCl3[3], which has ferromagnetic rung coupling. In order to clarify the mechanism of the two-step field-induced transition, we investigate the anisotropic spin ladder using the numerical diagonalization and the finite-size scaling analysis. As a result, we revealed that two different field-induced second-order quantum phase transitions possibly occur. Several phase diagrams are also presented. In addition we discuss on a possible two-step spin flop in other materials[4] and some frustrated systems. [1] C. N. Yang and C. P. Yang, Phys. Rev. 151 (1966) 258. [2] T. Sakai, Phys. Rev. B 58 (1998) 6268. [3] T. Masuda et al, Phys. Rev. Lett. 96 (2006) 047210. [4] H. Miyasaka et al, Inorg. Chem. 42 (2003) 8203.
Cooling into the spin-nematic state for a spin-1 Bose gas in an optical lattice
Chung, M.-C.; Yip Sungkit
2009-05-15
The possibility of adiabatically cooling a spin-1 polar Bose gas to a spin-nematic phase is theoretically discussed. The relation between the order parameter of the final spin-nematic phase and the starting temperature of the spinor Bose gas is obtained both using the mean-field approach for high temperature and spin-wave approach for low temperature. We find that there exists a good possibility to reach the spin-nematic ordering starting with spinor antiferromagnetic Bose gases.
Spin orbital theory for the high temperature magnetic phase transitions in Yttrium orthovanadate
NASA Astrophysics Data System (ADS)
de Silva, Theja; Joshi, Anuvrat; Zhang, Fu Chun; Ma, Michael
2003-03-01
Motivated by recent diffraction experiments, we develope a theoritical model for Yttrium orthovanadate(YVO_3). The key parameters governing the system are on-site coulomb repulsion, Hund's coupling, crystal field splitting between 3d levels and hopping amplitude between nearest neighbor ions. Then, we use a mean field theory to illustrate the relevent physics of the system and verify the existence of the high temperature G-type orbital transition before C-type spin ordering at a lower temperature.
Enhancement of spin accumulation in ballistic transport regime
NASA Astrophysics Data System (ADS)
Chen, Kai; Zhang, Shufeng
2015-12-01
The conventional spin-diffusion equation, based on the presence of spin-split local chemical potentials, has successfully described spin accumulation attendant to diffusive transport in spintronics. A recent experiment shows that spin accumulation far exceeds the limit set by such spin-diffusive theory when the mean free path is longer than the spin dephasing length. By introducing the momentum and spin dependent chemical potential, we develop a generalized spin transport equation that is capable of addressing spin transport in systems where ballistic processes are embedded in the overall diffusive conductor. We find that the ballistic spin injection through a barrier into a diffusive nonmagnetic layer with strong spin-orbit coupling can enhance spin accumulation by an order of magnitude when compared to the conventional theory.
Spin slush in an extended spin ice model
Rau, Jeffrey G.; Gingras, Michel J. P.
2016-01-01
We present a new classical spin liquid on the pyrochlore lattice by extending spin ice with further neighbour interactions. We find that this disorder-free spin model exhibits a form of dynamical heterogeneity with extremely slow relaxation for some spins, while others fluctuate quickly down to zero temperature. We thus call this state spin slush, in analogy to the heterogeneous mixture of solid and liquid water. This behaviour is driven by the structure of the ground-state manifold which extends the celebrated two-in/two-out ice states to include branching structures built from three-in/one-out, three-out/one-in and all-in/all-out tetrahedra defects. Distinctive liquid-like patterns in the magnetic correlations serve as a signature of this intermediate range order. Possible applications to materials as well the effects of quantum tunnelling are discussed. PMID:27470199
Spin slush in an extended spin ice model
NASA Astrophysics Data System (ADS)
Rau, Jeffrey G.; Gingras, Michel J. P.
2016-07-01
We present a new classical spin liquid on the pyrochlore lattice by extending spin ice with further neighbour interactions. We find that this disorder-free spin model exhibits a form of dynamical heterogeneity with extremely slow relaxation for some spins, while others fluctuate quickly down to zero temperature. We thus call this state spin slush, in analogy to the heterogeneous mixture of solid and liquid water. This behaviour is driven by the structure of the ground-state manifold which extends the celebrated two-in/two-out ice states to include branching structures built from three-in/one-out, three-out/one-in and all-in/all-out tetrahedra defects. Distinctive liquid-like patterns in the magnetic correlations serve as a signature of this intermediate range order. Possible applications to materials as well the effects of quantum tunnelling are discussed.
Spin slush in an extended spin ice model.
Rau, Jeffrey G; Gingras, Michel J P
2016-01-01
We present a new classical spin liquid on the pyrochlore lattice by extending spin ice with further neighbour interactions. We find that this disorder-free spin model exhibits a form of dynamical heterogeneity with extremely slow relaxation for some spins, while others fluctuate quickly down to zero temperature. We thus call this state spin slush, in analogy to the heterogeneous mixture of solid and liquid water. This behaviour is driven by the structure of the ground-state manifold which extends the celebrated two-in/two-out ice states to include branching structures built from three-in/one-out, three-out/one-in and all-in/all-out tetrahedra defects. Distinctive liquid-like patterns in the magnetic correlations serve as a signature of this intermediate range order. Possible applications to materials as well the effects of quantum tunnelling are discussed. PMID:27470199
NASA Astrophysics Data System (ADS)
Chau, N.; Tho, N. D.; Luong, N. H.; Giang, B. H.; Cong, B. T.
2006-08-01
The mixed rare earth manganites Nd 0.5-xPr xSr 0.5MnO 3 ( x=0.1-0.5) have been prepared using solid state reaction technique. All samples are of single phase with orthorhombic structure. The microstructure of the samples was determined by SEM. The field-cooled (FC) and zero-field-cooled (ZFC) curves showed that samples with x⩾0.25 exhibit the spin glass-like state at low field and low temperatures, whereas, in the samples with x<0.25, there is the charge ordering (coexisting with FM-AFM transition) established at low temperatures. The Curie temperature of the samples increases with increasing Pr content due to increase of < rA>. Interesting feature is that at the FM-AFM transition region, the magnetic entropy change has positive value, in contrary to that at FM-PM transition region. The electrical property of the samples from 10 K to room temperature is examined in detail.
Spectroscopy of composite solid-state spin environments for improved metrology with spin ensembles
NASA Astrophysics Data System (ADS)
Bar-Gill, Nir; Pham, Linh; Belthangady, Chinmay; Lesage, David; Cappellaro, Paola; Maze, Jeronimo; Lukin, Mikhail; Yacoby, Amir; Walsworth, Ronald
2012-02-01
For precision coherent measurements with ensembles of quantum spins the relevant Figure-of-Merit (FOM) is the product of spin density and coherence lifetime, which is generally limited by the dynamics of spin coupling to the environment. Significant effort has been invested in understanding the causes of decoherence in a diverse range of spin systems in order to increase the FOM and improve measurement sensitivity. Here, we apply a coherent spectroscopic technique to characterize the dynamics of a composite solid-state spin environment consisting of Nitrogen-Vacancy (NV) color centers in room temperature diamond coupled to baths of electronic spin (N) and nuclear spin (13C) impurities. For diamond samples with a wide range of NV densities and impurity spin concentrations we employ a dynamical decoupling technique to minimize coupling to the environment, and find similar values for the FOM, which is three orders of magnitude larger than previously achieved in any room-temperature solid-state spin system, and thus should enable greatly improved precision spin metrology. We also identify a suppression of electronic spin bath dynamics in the presence of a nuclear spin bath of sufficient nuclear spin concentration. This suppression could inform efforts to engineer samples with even larger FOM for solid-state spin ensemble metrology and collective quantum information processing.
Artificial frustrated spin systems
NASA Astrophysics Data System (ADS)
Perrin, Y.; Chioar, I. A.; Nguyen, V. D.; Lacour, D.; Hehn, M.; Montaigne, F.; Canals, B.; Rougemaille, N.
2015-09-01
Complex architectures of nanostructures are routinely elaborated using bottom-up or nanofabrication processes. This technological capability allows scientists to engineer materials with properties that do not exist in nature, but also to manufacture model systems to explore fundamental issues in condensed matter physics. Two-dimensional frustrated arrays of magnetic nanostructures are one class of systems for which theoretical predictions can be tested experimentally. These systems have been the subject of intense research in the last few years and allowed the investigation of a rich physics and fascinating phenomena, such as the exploration of the extensively degenerate ground-state manifolds of spin ice systems, the evidence of new magnetic phases in purely two-dimensional lattices, and the observation of pseudoexcitations involving classical analogues of magnetic monopoles. We show here, experimentally and theoretically, that simple magnetic geometries can lead to unconventional, non-collinear spin textures. For example, kagome arrays of inplane magnetized nano-islands do not show magnetic order. Instead, these systems are characterized by spin textures with intriguing properties, such as chirality, coexistence of magnetic order and disorder, and charge crystallization. Magnetic frustration effects in lithographically patterned kagome arrays of nanomagnets with out-of-plane magnetization also lead to an unusal, and still unknown, magnetic ground state manifold. Besides the influence of the lattice geometry, the micromagnetic nature of the elements constituting the arrays introduce the concept of chiral magnetic monopoles, bringing additional complexity into the physics of artificial frustrated spin systems.
35% magnetocurrent with spin transport through Si
NASA Astrophysics Data System (ADS)
Huang, Biqin; Zhao, Lai; Monsma, Douwe J.; Appelbaum, Ian
2007-07-01
Efficient injection of spin-polarized electrons into the conduction band of silicon is limited by the formation of a silicide at the ferromagnetic metal (FM)/silicon interface. In the present work, this "magnetically dead" silicide (where strong spin scattering significantly reduces injected spin polarization) is eliminated by moving the FM in the spin injector from the tunnel junction base anode to the emitter cathode and away from the silicon surface. This results in over an order-of-magnitude increase in spin injection efficiency, from a previously reported magnetocurrent ratio of ≈2% to ≈35% and an estimated spin polarization in Si from ≈1% to at least ≈15%. The injector tunnel junction bias dependence of this spin transport signal is also measured, demonstrating the importance of low bias voltage to preserve high injected spin polarization.
Dynamics of antiferromagnets driven by spin current
NASA Astrophysics Data System (ADS)
Cheng, Ran; Niu, Qian
2014-02-01
When a spin-polarized current flows through a ferromagnetic (FM) metal, angular momentum is transferred to the background magnetization via spin-transfer torques. In antiferromagnetic (AFM) materials, however, the corresponding problem is unsolved. We derive microscopically the dynamics of an AFM system driven by spin current generated by an attached FM polarizer, and find that the spin current exerts a driving force on the local staggered order parameter. The mechanism does not rely on the conservation of spin angular momentum, nor does it depend on the induced FM moments on top the AFM background. Two examples are studied: (i) A domain wall is accelerated to a terminal velocity by purely adiabatic effect where the Walker's breakdown is avoided. (ii) Spin injection modifies the AFM resonance frequency, and spin current injection triggers spin wave instability of local moments above a threshold.
Andersen, John A.; Flanigan, John J.; Kindley, Robert J.
1978-01-01
The disclosure relates to an apparatus for spin ejecting a body having a flat plate base containing bosses. The apparatus has a base plate and a main ejection shaft extending perpendicularly from the base plate. A compressible cylindrical spring is disposed about the shaft. Bearings are located between the shaft and the spring. A housing containing a helical aperture releasably engages the base plate and surrounds the shaft bearings and the spring. A piston having an aperture follower disposed in the housing aperture is seated on the spring and is guided by the shaft and the aperture. The spring is compressed and when released causes the piston to spin eject the body.
Spin liquid phases of large spin Mott insulating ultracold atoms
NASA Astrophysics Data System (ADS)
Rutkowski, Todd C.; Lawler, Michael J.
2015-03-01
Understanding exotic forms of magnetism, primarily those driven by large spin fluctuations such as the quantum spin liquid state, is a major goal of condensed matter physics. But, the relatively small number of viable candidate materials poses a difficulty. We believe this problem can be solved by Mott insulating ultracold atoms with large spin moments that interact via whole-atom exchange. The large spin fluctuations of this exchange could stabilize exotic physics similar to condensed matter systems, all in an extremely tunable environment. We have approached the problem by performing a mean field theory for spin-f bosons in an optical lattice which is exact in the large-f limit. This setting is similar to that of SU(N) magnetism proposed for alkali-earth atoms but without the SU(N) symmetry. We find that states with long-range order, such as the spin nematic phase of f = 1 Na atoms, become highly entangled spin-liquid-like states for f = 3 Cr atoms. This is evidence that the magnetic phase diagram for Mott insulating atoms at larger spins generically contains exotic forms of magnetism.
Spin pumping and inverse spin Hall effects in heavy metal/antiferromagnet/Permalloy trilayers
NASA Astrophysics Data System (ADS)
Saglam, Hilal; Zhang, Wei; Jungfleisch, M. Benjamin; Jiang, Wanjun; Pearson, John E.; Hoffmann, Axel
Recent work shows efficient spin transfer via spin waves in insulating antiferromagnets (AFMs), suggesting that AFMs can play a more active role in the manipulation of ferromagnets. We use spin pumping and inverse spin Hall effect experiments on heavy metal (Pt and W)/AFMs/Py (Ni80Fe20) trilayer structures, to examine the possible spin transfer phenomenon in metallic AFMs, i . e . , FeMn and PdMn. Previous work has studied electronic effects of the spin transport in these materials, yielding short spin diffusion length on the order of 1 nm. However, the work did not examine whether besides diffusive spin transport by the conduction electrons, there are additional spin transport contributions from spin wave excitations. We clearly observe spin transport from the Py spin reservoir to the heavy metal layer through the sandwiched AFMs with thicknesses well above the previously measured spin diffusion lengths, indicating that spin transport by spin waves may lead to non-negligible contributions This work was supported by US DOE, OS, Materials Sciences and Engineering Division. Lithographic patterning was carried out at the CNM, which is supported by DOE, OS under Contract No. DE-AC02-06CH11357.
Density and Spin Response Functions in Ultracold Fermionic Atom Gases
Mihaila, Bogdan; Blagoev, Krastan B.; Balatsky, Alexander V.; Smith, Darryl L.; Gaudio, Sergio; Littlewood, Peter B.
2005-08-26
We propose a new method of detecting the onset of superfluidity in a two-component ultracold fermionic gas of atoms governed by an attractive short-range interaction. By studying the two-body correlation functions we find that a measurement of the momentum distribution of the density and spin-response functions allows one to access separately the normal and anomalous densities. The change in sign at low momentum transfer of the normal-ordered part of the density response function signals the transition between a BEC and a BCS regime, characterized by small and large pairs, respectively. This change in sign of the density response function represents an unambiguous signature of the BEC-to-BCS crossover. Spin rotational symmetry breaking due to the magnetic field, if observed, can be used to validate the one-channel model.
Communication at the quantum speed limit along a spin chain
Murphy, Michael; Montangero, Simone; Giovannetti, Vittorio; Calarco, Tommaso
2010-08-15
Spin chains have long been considered as candidates for quantum channels to facilitate quantum communication. We consider the transfer of a single excitation along a spin-1/2 chain governed by Heisenberg-type interactions. We build on the work of Balachandran and Gong [V. Balachandran and J. Gong, Phys. Rev. A 77, 012303 (2008)] and show that by applying optimal control to an external parabolic magnetic field, one can drastically increase the propagation rate by two orders of magnitude. In particular, we show that the theoretical maximum propagation rate can be reached, where the propagation of the excitation takes the form of a dispersed wave. We conclude that optimal control is not only a useful tool for experimental application, but also for theoretical inquiry into the physical limits and dynamics of many-body quantum systems.
Numerical Modeling of the Central Spin Problem Using the Spin-Coherent-State P Representation
Al Hassanieh, Khaled A; Dobrovitski, V. V.; Dagotto, Elbio R; Harmon, B. N.
2006-01-01
In this work, we consider decoherence of a central spin by a spin bath. In order to study the nonperturbative decoherence regimes, we develop an efficient mean-field-based method for modeling the spin-bath decoherence, based on the P representation of the central spin density matrix. The method can be applied to longitudinal and transverse relaxation at different external fields. In particular, by modeling large-size quantum systems (up to 16 000 bath spins), we make controlled predictions for the slow long-time decoherence of the central spin.
Thermoelectric spin transport through ferromagnetic heterostructures
NASA Astrophysics Data System (ADS)
Bender, Scott A.
2015-10-01
We study how spin is transferred by ferromagnetic dynamics in a charge insulator in response to a thermoelectric bias, which is established by supplying heat and/or spin accumulation via normal leads. At zero temperature, magnetic anisotropies pin the macroscopic order, which necessitates a finite threshold bias to induce a spin current in a steady state of unpinned dynamics. At finite temperatures, however, thermal spin waves provide a spin transport channel in response to a linear thermoelectric bias. The theoretical description is rooted in the Landau-Lifshitz-Gilbert phenomenology both for the macroscopic dynamics of the magnetic order and quantum kinetics of thermal magnons. In this paper we connect the classical and quantum aspects of the underlying magnetic dynamics and spin transport, as well as provide a unified view of the exchange mediated bias of spin See-beck physics of the magnetic interface and bulk.
Montoncello, F.; Giovannini, L.; Nizzoli, F.; Vavassori, P.; Grimsditch, M.; Materials Science Division; Univ. di Ferrara; CNISM; CNR-INFM; CIC nanoGUNE Res. Ctr.
2008-06-01
We study the magnetization reversal in elliptical nanodots with the external field applied exactly along the minor (hard) axis. By varying the magnitude of the applied field, several first and second order transitions take place and the system proceeds through magnetic configurations characterized by different symmetry properties. The dynamical matrix method is used to calculate the spin excitations as function of the applied field. This model system allows us to investigate the relationship between the singularities of the magnetization, the presence of soft spin excitations, and the symmetry properties of the static and dynamic magnetization fields. Rules that govern the transitions are formulated.
Transverse target spin asymmetry in inclusive DIS with two-photon exchange
Afanasev, A.; Strikman, M.; Weiss, C.
2008-01-01
We study the transverse target spin dependence of the cross section for inclusive electron-nucleon scattering with unpolarized beam. Such dependence is absent in the one-photon exchange approximation (Christ-Lee theorem) and arises only in higher orders of the QED expansion, from the interference of one-photon and absorptive two-photon exchange amplitudes as well as from real photon emission (bremsstrahlung). We demonstrate that the transverse spin-dependent two-photon exchange cross section is free of QED infrared and collinear divergences. We argue that in DIS kinematics the transverse spin dependence should be governed by a 'partonlike' mechanism in which the two-photon exchange couples mainly to a single quark. We calculate the normal spin asymmetry in an approximation where the dominant contribution arises from quark-helicity flip due to interactions with nonperturbative vacuum fields (constituent quark picture) and is proportional to the quark transversity distribution in the nucleon. Such helicity-flip processes are not significantly Sudakov-suppressed if the infrared scale for gluon emission in the photon-quark subprocess is of the order of the chiral symmetry breaking scale, {mu}{sub chiral}{sup 2}>>{lambda}{sub QCD}{sup 2}. We estimate the asymmetry in the kinematics of the planned Jefferson Lab Hall A experiment to be of the order 10{sup -4}, with different sign for proton and neutron. We also comment on the spin dependence in the limit of soft high-energy scattering.
Transverse target spin asymmetry in inclusive DIS with two-photon exchange
NASA Astrophysics Data System (ADS)
Afanasev, A.; Strikman, M.; Weiss, C.
2008-01-01
We study the transverse target spin dependence of the cross section for inclusive electron-nucleon scattering with unpolarized beam. Such dependence is absent in the one-photon exchange approximation (Christ-Lee theorem) and arises only in higher orders of the QED expansion, from the interference of one-photon and absorptive two-photon exchange amplitudes as well as from real photon emission (bremsstrahlung). We demonstrate that the transverse spin-dependent two-photon exchange cross section is free of QED infrared and collinear divergences. We argue that in DIS kinematics the transverse spin dependence should be governed by a “partonlike” mechanism in which the two-photon exchange couples mainly to a single quark. We calculate the normal spin asymmetry in an approximation where the dominant contribution arises from quark-helicity flip due to interactions with nonperturbative vacuum fields (constituent quark picture) and is proportional to the quark transversity distribution in the nucleon. Such helicity-flip processes are not significantly Sudakov-suppressed if the infrared scale for gluon emission in the photon-quark subprocess is of the order of the chiral symmetry breaking scale, μchiral2≫ΛQCD2. We estimate the asymmetry in the kinematics of the planned Jefferson Lab Hall A experiment to be of the order 10-4, with different sign for proton and neutron. We also comment on the spin dependence in the limit of soft high-energy scattering.
Transverse target spin asymmetry in inclusive DIS with two-photon exchange
Andrei Afanasev; Mark Strikman; Christian Weiss
2007-09-06
We study the transverse target spin dependence of the cross section for the inclusive electron-nucleon scattering with unpolarized beam. Such dependence is absent in the one-photon exchange approximation (Christ-Lee theorem) and arises only in higher orders of the QED expansion, from the interference of one-photon and absorptive two-photon exchange amplitudes as well as from real photon emission (bremsstrahlung). We demonstrate that the transverse spin-dependent two-photon exchange cross section is free of QED infrared and collinear divergences. We argue that in DIS kinematics the transverse spin dependence should be governed by a "parton-like" mechanism in which the two-photon exchange couples mainly to a single quark. We calculate the normal spin asymmetry in an approximation where the dominant contribution arises from quark helicity flip due to interactions with non-perturbative vacuum fields (constituent quark picture) and is proportional to the quark transversity distribution in the nucleon. Such helicity-flip processes are not significantly Sudakov-suppressed if the infrared scale for gluon emission in the photon-quark subprocess is of the order of the chiral symmetry breaking scale, mu^2_chiral>>Lambda^2_QCD. We estimate the asymmetry in the kinematics of the planned Jefferson Lab Hall A experiment to be of the order 10^-4, with different sign for proton and neutron. We also comment on the spin dependence in the limit of soft high-energy scattering.
Spin-transfer torques in helimagnets
NASA Astrophysics Data System (ADS)
Hals, Kjetil M. D.; Brataas, Arne
2013-05-01
We theoretically investigate current-induced magnetization dynamics in chiral-lattice helimagnets. Spin-orbit coupling in noncentrosymmetric crystals induces a reactive spin-transfer torque that has not been previously considered. We demonstrate how the torque is governed by the crystal symmetry and acts as an effective magnetic field along the current direction in cubic B20-type crystals. The effects of the new torque are computed for current-induced dynamics of spin spirals and the Doppler shift of spin waves. In current-induced spin-spiral motion, the new torque tilts the spiral structure. The spin waves of the spiral structure are initially displaced by the new torque, while the dispersion relation is unaffected.
Random SU(2)-symmetric spin-S chains
NASA Astrophysics Data System (ADS)
Quito, V. L.; Hoyos, José A.; Miranda, E.
2016-08-01
We study the low-energy physics of a broad class of time-reversal invariant and SU(2)-symmetric one-dimensional spin-S systems in the presence of quenched disorder via a strong-disorder renormalization-group technique. We show that, in general, there is an antiferromagnetic phase with an emergent SU (2 S +1 ) symmetry. The ground state of this phase is a random singlet state in which the singlets are formed by pairs of spins. For integer spins, there is an additional antiferromagnetic phase which does not exhibit any emergent symmetry (except for S =1 ). The corresponding ground state is a random singlet one but the singlets are formed mostly by trios of spins. In each case the corresponding low-energy dynamics is activated, i.e., with a formally infinite dynamical exponent, and related to distinct infinite-randomness fixed points. The phase diagram has two other phases with ferromagnetic tendencies: a disordered ferromagnetic phase and a large spin phase in which the effective disorder is asymptotically finite. In the latter case, the dynamical scaling is governed by a conventional power law with a finite dynamical exponent.
Spin Technologies in Silicon Carbide
NASA Astrophysics Data System (ADS)
Klimov, Paul
2015-03-01
Over the past several decades SiC has evolved from being a simple abrasive to a versatile material platform for high-power electronics, optoelectronics, and nanomechanical devices. These technologies have been driven by advanced growth, doping, and processing capabilities, and the ready availability of large-area, single-crystal SiC wafers. Recent advances have also established SiC as a promising host for a novel class of technologies based on the spin of intrinsic color centers. In particular, the divacancies and related defects have ground-state electronic-spin triplets with ms-long coherence times that can be optically addressed near telecom wavelengths and manipulated with magnetic, electric, and strain fields. Recently, divacancy addressability has been extended to the single defect level, laying foundation for single spin technologies in SiC. This rapidly developing field has prompted research into the SiC material host to understand how defect-bound electron spins interact with their surrounding nuclear spin bath. Although nuclear spins are typically a major source of decoherence in color-center spin systems, they are also an important resource since they interact with magnetic fields orders of magnitude more weakly than electronic spins. This fact has motivated their use for quantum memories and ultra-sensitive sensors. In this talk I will review advances in this rapidly developing field and discuss our efforts towards this latter goal. This work was supported by the AFOSR, DARPA, and the NSF.
Spin Gradient Demagnetization Cooling of Ultracold Atoms
Medley, Patrick; Weld, David M.; Miyake, Hirokazu; Pritchard, David E.; Ketterle, Wolfgang
2011-05-13
We demonstrate a new cooling method in which a time-varying magnetic field gradient is applied to an ultracold spin mixture. This enables preparation of isolated spin distributions at positive and negative effective spin temperatures of {+-}50 pK. The spin system can also be used to cool other degrees of freedom, and we have used this coupling to cool an apparently equilibrated Mott insulator of rubidium atoms to 350 pK. These are the lowest temperatures ever measured in any system. The entropy of the spin mixture is in the regime where magnetic ordering is expected.
Lagrangian geometrical optics of nonadiabatic vector waves and spin particles
NASA Astrophysics Data System (ADS)
Ruiz, D. E.; Dodin, I. Y.
2015-10-01
Linear vector waves, both quantum and classical, experience polarization-driven bending of ray trajectories and polarization dynamics that can be interpreted as the precession of the "wave spin". Both phenomena are governed by an effective gauge Hamiltonian vanishing in leading-order geometrical optics. This gauge Hamiltonian can be recognized as a generalization of the Stern-Gerlach Hamiltonian that is commonly known for spin-1/2 quantum particles. The corresponding reduced Lagrangians for continuous nondissipative waves and their geometrical-optics rays are derived from the fundamental wave Lagrangian. The resulting Euler-Lagrange equations can describe simultaneous interactions of N resonant modes, where N is arbitrary, and lead to equations for the wave spin, which happens to be an (N2 - 1)-dimensional spin vector. As a special case, classical equations for a Dirac particle (N = 2) are deduced formally, without introducing additional postulates or interpretations, from the Dirac quantum Lagrangian with the Pauli term. The model reproduces the Bargmann-Michel-Telegdi equations with added Stern-Gerlach force.
Lagrangian geometrical optics of nonadiabatic vector waves and spin particles
Ruiz, D. E.; Dodin, I. Y.
2015-07-29
Linear vector waves, both quantum and classical, experience polarization-driven bending of ray trajectories and polarization dynamics that can be interpreted as the precession of the "wave spin". Here, both phenomena are governed by an effective gauge Hamiltonian vanishing in leading-order geometrical optics. This gauge Hamiltonian can be recognized as a generalization of the Stern-Gerlach Hamiltonian that is commonly known for spin-1/2 quantum particles. The corresponding reduced Lagrangians for continuous nondissipative waves and their geometrical-optics rays are derived from the fundamental wave Lagrangian. The resulting Euler-Lagrange equations can describe simultaneous interactions of N resonant modes, where N is arbitrary, and lead to equations for the wave spin, which happens to be an (N^{2} - 1)-dimensional spin vector. As a special case, classical equations for a Dirac particle (N = 2) are deduced formally, without introducing additional postulates or interpretations, from the Dirac quantum Lagrangian with the Pauli term. The model reproduces the Bargmann-Michel-Telegdi equations with added Stern-Gerlach force.
Lagrangian geometrical optics of nonadiabatic vector waves and spin particles
Ruiz, D. E.; Dodin, I. Y.
2015-10-01
Linear vector waves, both quantum and classical, experience polarization-driven bending of ray trajectories and polarization dynamics that can be interpreted as the precession of the "wave spin". Both phenomena are governed by an effective gauge Hamiltonian vanishing in leading-order geometrical optics. This gauge Hamiltonian can be recognized as a generalization of the Stern-Gerlach Hamiltonian that is commonly known for spin-1/2 quantum particles. The corresponding reduced Lagrangians for continuous nondissipative waves and their geometrical-optics rays are derived from the fundamental wave Lagrangian. The resulting Euler-Lagrange equations can describe simultaneous interactions of N resonant modes, where N is arbitrary, and lead to equations for the wave spin, which happens to be an (N-2 - 1)-dimensional spin vector. As a special case, classical equations for a Dirac particle (N = 2) are deduced formally, without introducing additional postulates or interpretations, from the Dirac quantum Lagrangian with the Pauli term. The model reproduces the Bargmann-Michel-Telegdi equations with added Stern-Gerlach force. (C) 2015 Elsevier B.V. All rights reserved.
Lagrangian geometrical optics of nonadiabatic vector waves and spin particles
Ruiz, D. E.; Dodin, I. Y.
2015-07-29
Linear vector waves, both quantum and classical, experience polarization-driven bending of ray trajectories and polarization dynamics that can be interpreted as the precession of the "wave spin". Here, both phenomena are governed by an effective gauge Hamiltonian vanishing in leading-order geometrical optics. This gauge Hamiltonian can be recognized as a generalization of the Stern-Gerlach Hamiltonian that is commonly known for spin-1/2 quantum particles. The corresponding reduced Lagrangians for continuous nondissipative waves and their geometrical-optics rays are derived from the fundamental wave Lagrangian. The resulting Euler-Lagrange equations can describe simultaneous interactions of N resonant modes, where N is arbitrary, and leadmore » to equations for the wave spin, which happens to be an (N2 - 1)-dimensional spin vector. As a special case, classical equations for a Dirac particle (N = 2) are deduced formally, without introducing additional postulates or interpretations, from the Dirac quantum Lagrangian with the Pauli term. The model reproduces the Bargmann-Michel-Telegdi equations with added Stern-Gerlach force.« less
Hanson, D.J.; Lepkowski, W.; Long, J.R.; Zurer, P.S.
1993-10-11
Both Clinton and Vice President Al Gore are committed to reinventing the federal government. To do so they will need more than a little help from Congress. But, if they succeed in turning the report's recommendations into reality, substantial change will occur in the way the federal government interacts with the chemical community in areas such as environmental and safety and health regulation, science and technology policy, education, and research priority setting. The report is the result of a six-month effort by the National Performance Review (NPR), a group led by Gore. It contains some 400 specific recommendations for changing the ways the federal government operates. These recommendations, if enacted the report claims, would produced savings of $108 billion over five years and reduce the size of the civilian, nonpostal work force by 12%, 252 positions, over the same period. The Department of Energy is the target of eight NPR recommendations. But the one with the most direct relevance to R and D calls for directing its national laboratories to pursue post-Cold War research priorities. Efforts to shift the labs away from their defense orientation began during the Carter presidency, when all of the labs began establishing stronger research programs in environmental science and technology and biology.
Spin Orbit Interaction Engineering for beyond Spin Transfer Torque memory
NASA Astrophysics Data System (ADS)
Wang, Kang L.
Spin transfer torque memory uses electron current to transfer the spin torque of electrons to switch a magnetic free layer. This talk will address an alternative approach to energy efficient non-volatile spintronics through engineering of spin orbit interaction (SOC) and the use of spin orbit torque (SOT) by the use of electric field to improve further the energy efficiency of switching. I will first discuss the engineering of interface SOC, which results in the electric field control of magnetic moment or magneto-electric (ME) effect. Magnetic memory bits based on this ME effect, referred to as magnetoelectric RAM (MeRAM), is shown to have orders of magnitude lower energy dissipation compared with spin transfer torque memory (STTRAM). Likewise, interests in spin Hall as a result of SOC have led to many advances. Recent demonstrations of magnetization switching induced by in-plane current in heavy metal/ferromagnetic heterostructures have been shown to arise from the large SOC. The large SOC is also shown to give rise to the large SOT. Due to the presence of an intrinsic extraordinarily strong SOC and spin-momentum lock, topological insulators (TIs) are expected to be promising candidates for exploring spin-orbit torque (SOT)-related physics. In particular, we will show the magnetization switching in a chromium-doped magnetic TI bilayer heterostructure by charge current. A giant SOT of more than three orders of magnitude larger than those reported in heavy metals is also obtained. This large SOT is shown to come from the spin-momentum locked surface states of TI, which may further lead to innovative low power applications. I will also describe other related physics of SOC at the interface of anti-ferromagnetism/ferromagnetic structure and show the control exchange bias by electric field for high speed memory switching. The work was in part supported by ERFC-SHINES, NSF, ARO, TANMS, and FAME.
Spin pumping and spin Seebeck effect
NASA Astrophysics Data System (ADS)
Saitoh, Eiji
2012-02-01
Utilization of a spin current, a flow of electrons' spins in a solid, is the key technology in spintronics that will allow the achievement of efficient magnetic memories and computing devices. In this technology, generation and detection of spin currents are necessary. Here, we review inverse spin-Hall effect and spin-current-generation phenomena recently discovered both in metals and insulators: inverse spin-Hall effect, spin pumping, and spin Seebeck effect. (1)Spin pumping and spin torque in a Mott insulator system We found that spin pumping and spin torque effects appear also at an interface between Pt and an insulator YIG.. This means that we can connect a spin current carried by conduction electrons and a spin-wave spin current flowing in insulators. We demonstrate electric signal transmission by using these effects and interconversion of the spin currents [1]. (2) Spin Seebeck effect We have observed, by using the inverse spin-Hall effect [2], spin voltage generation from a heat current in a NiFe, named the spin-Seebeck effect [3]. Surprisingly, spin-Seebeck effect was found to appear even in insulators [4], a situation completely different from conventional charge Seebeck effect. The result implies an important role of elementary excitation in solids beside charge in the spin Seebeck effect. In the talk, we review the recent progress of the research on this effect. This research is collaboration with K. Ando, K. Uchida, Y. Kajiwara, S. Maekawa, G. E. W. Bauer, S. Takahashi, and J. Ieda. [4pt] [1] Y. Kajiwara and E. Saitoh et al. Nature 464 (2010) 262. [0pt] [2] E. Saitoh et al., Appl. Phys. Lett. 88 (2006) 182509. [0pt] [3] K. Uchida and E. Saitoh et al., Nature 455 (2008)778. [0pt] [4] K. Uchida and E. Saitoh et al.,Nature materials 9 (2010) 894 - 897.
Suppression of spin-exchange relaxation in tilted magnetic fields within the geophysical range
NASA Astrophysics Data System (ADS)
Scholtes, Theo; Pustelny, Szymon; Fritzsche, Stephan; Schultze, Volkmar; Stolz, Ronny; Meyer, Hans-Georg
2016-07-01
We present a detailed experimental and theoretical study on the relaxation of spin coherence due to the spin-exchange mechanism arising in the electronic ground states of alkali-metal vapor atoms. As opposed to the well-explored formation of a stretched state in a longitudinal geometry (magnetic field parallel to the laser propagation direction) we employ adapted hyperfine-selective optical pumping in order to suppress spin-exchange relaxation. By comparing measurements of the intrinsic relaxation rate of the spin coherence in the ground state of cesium atoms with detailed density-matrix simulations we show that the relaxation due to spin-exchange collisions can be reduced substantially even in a tilted magnetic field of geomagnetic strength, the major application case of scalar magnetic surveying. This explains the observed striking improvement in sensitivity and further deepens the understanding of the light-narrowed Mx magnetometer, which was presented recently. Additionally, new avenues for investigating the dynamics in alkali-metal atoms governed by the spin-exchange interaction and interacting with arbitrary external fields open up.
Observation of two-orbital spin-exchange interactions with ultracold SU(N)-symmetric fermions
NASA Astrophysics Data System (ADS)
Scazza, F.; Hofrichter, C.; Höfer, M.; de Groot, P. C.; Bloch, I.; Fölling, S.
2014-10-01
Spin-exchanging interactions govern the properties of strongly correlated electron systems such as many magnetic materials. When orbital degrees of freedom are present, spin exchange between different orbitals often dominates, leading to the Kondo effect, heavy fermion behaviour or magnetic ordering. Ultracold ytterbium or alkaline-earth ensembles have attracted much recent interest as model systems for these effects, with two (meta-) stable electronic configurations representing independent orbitals. We report the observation of spin-exchanging contact interactions in a two-orbital SU(N)-symmetric quantum gas realized with fermionic 173Yb. We find strong inter-orbital spin exchange by spectroscopic characterization of all interaction channels and demonstrate SU(N = 6) symmetry within our measurement precision. The spin-exchange process is also directly observed through the dynamic equilibration of spin imbalances between ensembles in separate orbitals. The realization of an SU(N)-symmetric two-orbital Hubbard Hamiltonian opens the route to quantum simulations with extended symmetries and with orbital magnetic interactions, such as the Kondo lattice model.
Novel effects of spin-orbit interaction in interacting electronic systems
NASA Astrophysics Data System (ADS)
Sun, Jianmin
Over the last several years there has been a remarkable growth in research activity in the physical properties of mesoscopic systems. Significant results, which were obtained by both theoretical and experimental studies, together with the enormous promise of nano-technology applications, contribute to this interest. In mesoscopic systems, there are 1023 or so electrons with strong Coulomb interaction. The length scale governing the electrons motion is small enough to cause quantization of the energy levels. In this work we study such quantum systems: quantum wires, quantum dots. During the last decade several experimental techniques have been developed for manufacturing both kinds of devices, which are currently an important tool for understanding low dimensions physics. The finite spin-orbit coupling is very natural, and, strictly speaking, unavoidable, in semiconducting quantum wires due to pronounced structural asymmetry inherent in the fabrication process. Thus the interplay between Coulomb interaction and spin-orbit coupling is important to investigate. The magnetic field also plays an important role which breaks the time-reversal symmetry of the Hamiltonian and splits the band of free electrons into two, corresponding to up-spin and down-spin electrons, reducing spin-rotational symmetry of the system from SU(2) to U(1). The dissertation takes account of the effect of the spin-orbit coupling interactions in the properties of mesoscopic systems. The manuscript is divided in four Chapters. In Chapter 1, the field theory in mesoscopic system is introduced. I present the relations between bosonic and fermionic operators in one dimension. These relations are used to bosonize spin 1/2 interaction fermion system. I show how to derive the RG equations around a fixed-point from the Operator Product Expansion (OPE). In Chapter 2, I present analysis of the interacting quantum wire problem in the presence of magnetic field and spin-orbital interaction. I show that an
Creutz, Michael
2014-03-15
Quantum mechanics and relativity in the continuum imply the well known spin–statistics connection. However for particles hopping on a lattice, there is no such constraint. If a lattice model yields a relativistic field theory in a continuum limit, this constraint must “emerge” for physical excitations. We discuss a few models where a spin-less fermion hopping on a lattice gives excitations which satisfy the continuum Dirac equation. This includes such well known systems such as graphene and staggered fermions. -- Highlights: •The spin–statistics theorem is not required for particles on a lattice. •Spin emerges dynamically when spinless fermions have a relativistic continuum limit. •Graphene and staggered fermions are examples of this phenomenon. •The phenomenon is intimately tied to chiral symmetry and fermion doubling. •Anomaly cancellation is a crucial feature of any valid lattice fermion action.
Optical effects of spin currents in semiconductors
NASA Astrophysics Data System (ADS)
Wang, Jing
2011-03-01
BANG-FEN ZHU, Department of Physics and Institute of Advanced Study, Tsinghua University, REN-BAO LIU, Department of Physics, The Chinese University of Hong Kong -- We predict the linear and second-order nonlinear optical effects of spin currents in semiconductors, based on systematic symmetry analysis and microscopic calculations with realistic models [1, 2]. By an analogue to the Ampere effect and Oersted effect, we conceived and verified that a spin current can be coupled to a ``photon spin curren'' carried by a polarized light beam, which causes sizeable Faraday rotation without involving net magnetization. Furthermore, a spin current can have a strong second-order nonlinear optical effect with unique polarization-dependence due to the special symmetry properties of the spin current. In particular, for a longitudinal spin current, in which the spins point parallel or anti-parallel to the current direction is a chiral quantity, a chiral sum-frequency effect will be induced. The second-order optical effects of spin currents have been experimentally verified immediately after the theoretical prediction. These discoveries represent new phenomena in magneto-optics, with potential spin-photonic applications. They bring new opportunities to research of spintronics and may also facilitate research of topological insulators where the edge states form pure spin currents. This work was supported by the NSFC Grant Nos.10574076, 10774086, and the Basic Research Program of China Grant 2006CB921500, Hong Kong RGC HKU 10/CRF/08 and Hong Kong GRF CUHK 402207.
Moderate Positive Spin Hall Angle in Uranium
NASA Astrophysics Data System (ADS)
Anguera, Marta; Singh, Simran; Del Barco, Enrique; Springell, Ross; Miller, Casey W.
We will present results on FMR and voltage measurements of magnetic damping and the inverse spin Hall effect, respectively, in Ni80Fe20/Uranium bilayers. A pure spin current is injected into an Uranium film from the ferromagnetic resonance dynamics of the magnetization of an adjacent Ni80Fe20 (permalloy) film. The spin current generated is then converted into an electric field by the inverse spin Hall effect. Our results suggest a spin mixing conductance of order 2x1019 m-2 and a positive spin Hall angle of 0.004, which are both unexpected based on trends in d-electron systems. These results support the idea that materials with unfilled f-electron orbitals may require additional exploration for spin physics. Work at UCF was supported by NSF-ECCS grant # 1402990. Work at RIT was supported by NSF-ECCS Grant 1515677.
Radiation-spin interaction, Gilbert damping, and spin torque.
Ho, Jeongwon; Khanna, F C; Choi, B C
2004-03-01
Magnetization relaxation processes, which are represented by the Gilbert damping term and the spin torque term in the Landau-Lifshitz-Gilbert (LLG) equation, are described by the radiation-spin interaction (RSI), where the radiation field is produced by magnetization precessional motion itself. It is shown that the LLG equation including the Gilbert damping term and the spin torque term is derived from the spin Hamiltonian containing the RSI. The derivation of the LLG equation is given in a self-consistent method. It is also shown that, according to RSI, the magnitude of the magnetization vector deviates from the magnetization saturation with the order of O(alpha(2)), where alpha is the Gilbert damping parameter. PMID:15089513
Spinning compact binary dynamics and chameleon orbits
NASA Astrophysics Data System (ADS)
Gergely, László Árpád; Keresztes, Zoltán
2015-01-01
We analyze the conservative evolution of spinning compact binaries to second post-Newtonian (2PN) order accuracy, with leading-order spin-orbit, spin-spin and mass quadrupole-monopole contributions included. As a main result we derive a closed system of first-order differential equations in a compact form, for a set of dimensionless variables encompassing both orbital elements and spin angles. These evolutions are constrained by conservation laws holding at 2PN order. As required by the generic theory of constrained dynamical systems we perform a consistency check and prove that the constraints are preserved by the evolution. We apply the formalism to show the existence of chameleon orbits, whose local, orbital parameters evolve from elliptic (in the Newtonian sense) near pericenter, towards hyperbolic at large distances. This behavior is consistent with the picture that general relativity predicts stronger gravity at short distances than Newtonian theory does.
A new spin on electron liquids: Phenomena in systems with spin-orbit coupling
NASA Astrophysics Data System (ADS)
Bernevig, B. Andrei
Conventional microelectronic devices are based on the ability to store and control the flow of electronic charge. Spin-based electronics promises a radical alternative, offering the possibility of logic operations with much lower power consumption than equivalent charge-based logic operations. Our research suggests that spin transport is fundamentally different from the transport of charge. The generalized Ohm's law that governs the flow of spins indicates that the generation of spin current by an electric field can be reversible and non-dissipative. Spin-orbit coupling and spin currents appear in many other seemingly unrelated areas of physics. Spin currents are as fundamental in theoretical physics as charge currents. In strongly correlated systems such as spin-chains, one can write down the Hamiltonian as a spin-current - spin-current interaction. The research presented here shows that the fractionalized excitations of one-dimensional spin chains are gapless and carry spin current. We present the most interesting example of such a chain, the Haldane-Shastry spin chain, which is exactly solvable in terms of real-space wavefunctions. Spin-orbit coupling can be found in high-energy physics, hidden under a different name: non-trivial fibrations. Particles moving in a space which is non-trivially related to an (iso)spin space acquire a gauge connection (the condensed-matter equivalent of a Berry phase) which can be either abelian or non-abelian. In most cases, the consequences of such gauge connection are far-reaching. We present a problem where particles move on an 8-dimensional manifold and posses an isospin space with is a 7-sphere S 7. The non-trivial isospin space gives the Hamiltonian SO (8) landau-level structure, and the system exhibits a higher-dimensional Quantum Hall Effect.
Spin wave resonance detection using magnetic tunnel junction structure
NASA Astrophysics Data System (ADS)
Bi, Chong; Fan, Xin; Pan, Liqing; Kou, Xiaoming; Wu, Jun; Yang, Qinghui; Zhang, Huaiwu; Xiao, John Q.
2011-11-01
We have demonstrated that spin wave resonance in a permalloy microstrip can be detected by an electrical method based on magnetic tunnel junction structures. The detection method promises high spatial resolution and sensitivity. Both even and odd spin wave resonance modes can be clearly observed in a permalloy microstrip. The spin wave induced voltage is proportional to the input microwave power at each resonance mode. Data analysis using the model of quantized dipole-exchange spin wave resonance suggests the edge pinning of spin wave sensitively depends on the order of the spin wave mode, as well as on the excitation frequency for modes of the higher order.
Fluorine Functionalized BNNT as a Spin Filter
NASA Astrophysics Data System (ADS)
Dhungana, Kamal; Pati, Ranjit
2015-03-01
Spin filtering is a phenomenon that allows one to generate spin-polarized carriers in a circuit comprised of a magnetic channel sandwiched between two non-magnetic electrodes. In recent years, the quest for a novel low-dimensional metal-free magnetic channel that would exhibit both magnetism at a higher temperature and excellent spin filtering property has been intensively pursued. Herein, using a first-principles approach, we study the magnetic property of fluorine functionalized boron nitride nanotube (F-BNNT). A long range ferromagnetic spin ordering is found to occur in the F-BNNT at temperature much above the room temperature. Our spin polarized transport study shows that the fluorine functionalization in BNNT not only enhances its conductance by more than two orders, which is in excellent agreement with the experimental report, but also makes it a perfect spin filter. This work is supported by the NSF through Grant No. 1249504.
Paramagnetic and Antiferromagnetic Spin Seebeck Effect
NASA Astrophysics Data System (ADS)
Wu, Stephen
We report on the observation of the longitudinal spin Seebeck effect in both antiferromagnetic and paramagnetic insulators. By using a microscale on-chip local heater, it is possible to generate a large thermal gradient confined to the chip surface without a large increase in the total sample temperature. This technique allows us to easily access low temperatures (200 mK) and high magnetic fields (14 T) through conventional dilution refrigeration and superconducting magnet setups. By exploring this regime, we detect the spin Seebeck effect through the spin-flop transition in antiferromagnetic MnF2 when a large magnetic field (>9 T) is applied along the easy axis direction. Using the same technique, we are also able to resolve a spin Seebeck effect from the paramagnetic phase of geometrically frustrated antiferromagnet Gd3Ga5O12 (gadolinium gallium garnet) and antiferromagnetic DyScO3 (DSO). Since these measurements occur above the ordering temperatures of these two materials, short-range magnetic order is implicated as the cause of the spin Seebeck effect in these systems. The discovery of the spin Seebeck effect in these two materials classes suggest that both antiferromagnetic spin waves and spin excitations from short range magnetic order may be used to generate spin current from insulators and that the spin wave spectra of individual materials are highly important to the specifics of the longitudinal spin Seebeck effect. Since insulating antiferromagnets and paramagnets are far more common than the typical insulating ferrimagnetic materials used in spin Seebeck experiments, this discovery opens up a large new class of materials for use in spin caloritronic devices. All authors acknowledge support of the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division. The use of facilities at the Center for Nanoscale Materials, was supported by the U.S. DOE, BES under Contract No. DE-AC02-06CH11357.
Dynamical aspects of spin chains at infinite temperature for different spin quantum numbers
NASA Astrophysics Data System (ADS)
Böhm, Markus; Leschke, Hajo
1993-10-01
For infinite temperature we exactly calculate the coefficients of the short-time expansion of the spin-pair correlations in one-dimensional spin models. For spin quantum numbers s = 1 we present the coefficients up to order t18 and t22, for classical spins up to order t16 and t18 for the isotropic Heisenberg chain and the isotropic XY-chain, respectively. These coefficients are used together with recently determined ones for s = {1}/{2} to compute bounds on the autocorrelation functions, to approximate the associated spectral densities and to bound the spatial variances of pair correlations. The results are compared with those obtained from simulation data of Gerling and Landau (Phys. Rev. B 42 (1990) 8214) for classical spin chains. Over the available time region, we find a rather smooth dependence of the dynamics on the spin quantum number and see some evidence for spin diffusion.
Chiral projected entangled-pair state with topological order
NASA Astrophysics Data System (ADS)
Yang, Shuo; Wahl, Thorsten; Tu, Hong-Hao; Schuch, Norbert; Cirac, J. Ignacio
We show that projected entangled-pair states (PEPS) can describe chiral topologically ordered phases. For that, we construct a simple PEPS for spin-1/2 particles in a two-dimensional lattice. We reveal a symmetry in the local projector of the PEPS that gives rise to the global topological character. We also extract characteristic quantities of the edge conformal field theory using the bulk-boundary correspondence. EU projects SIQS and QALGO, the Alexander von Humboldt foundation, the Government of Canada through Industry Canada, and the Province of Ontario through the Ministry of Economic Development & Innovation.
Interaction-driven exotic quantum phases in spin-orbit-coupled spin-1 bosons
NASA Astrophysics Data System (ADS)
Pixley, J. H.; Natu, Stefan S.; Spielman, I. B.; Das Sarma, S.
2016-02-01
We study the interplay between large-spin, spin-orbit coupling, and superfluidity for bosons in a two-dimensional optical lattice, focusing on the spin-1 spin-orbit-coupled system recently realized at the Joint Quantum Institute [Campbell et al., arXiv:1501.05984]. We find a rich quantum phase diagram where, in addition to the conventional phases—superfluid and insulator—contained in the spin-1 Bose-Hubbard model, there are new lattice symmetry breaking phases. For weak interactions, the interplay between two length scales, the lattice momentum and the spin-orbit wave vector, induce a phase transition from a uniform superfluid to a phase where bosons simultaneously condense at the center and edge of the Brillouin zone at a nonzero spin-orbit strength. This state is characterized by spin-density-wave order, which arises from the spin-1 nature of the system. Interactions suppress spin-density-wave order, and favor a superfluid only at the Brillouin zone edge. This state has spatially oscillating mean-field order parameters, but a homogeneous density. We show that the spin-density-wave superfluid phase survives in a two-dimensional harmonic trap, and thus establish that our results are directly applicable to experiments on 87Rb,7Li, and 41K.
NASA Astrophysics Data System (ADS)
Piegsa, Florian M.; Hautle, Patrick; Schanzer, Christian
2016-04-01
A novel neutron spin resonance technique is presented based on the well-known neutron spin echo method. In a first proof-of-principle measurement using a monochromatic neutron beam, it is demonstrated that relative velocity changes of down to a precision of 4 ×10-7 can be resolved, corresponding to an energy resolution of better than 3 neV. Currently, the sensitivity is only limited by counting statistics and not by systematic effects. An improvement by another two orders of magnitude can be achieved with a dedicated setup, allowing energy resolutions in the 10 peV regime. The new technique is ideally suited for investigations in the field of precision fundamental neutron physics, but will also be beneficial in scattering applications.
Zadrozny, Joseph M; Graham, Michael J; Krzyaniak, Matthew D; Wasielewski, Michael R; Freedman, Danna E
2016-08-01
A counterintuitive three-order of magnitude slowing of the spin-lattice relaxation rate is observed in a high spin qubit at high magnetic field via multifrequency pulsed electron paramagnetic resonance measurements. PMID:27463410
Relativistic spin effects in the baryon spectrum
Garcilazo, Humberto
2005-04-01
We study the nonstrange baryon spectrum within a three-body theory that treats relativistically both the space and the spin variables. The relativistic effects of the spin are about one order of magnitude smaller than those due to the use of relativistic momentum variables. The relativistic treatment of the spin breaks the degenerancy that is present in the nonrelativistic model and in the model with only relativistic momentum variables.
Spin-2 particles in gravitational fields
Papini, G.
2007-02-15
We give a solution of the wave equation for massless, or massive spin-2 particles propagating in a gravitational background. The solution is covariant, gauge-invariant and exact to first order in the background gravitational field. The background contribution is confined to a phase factor from which geometrical and physical optics can be derived. The phase also describes Mashhoon's spin-rotation coupling and, in general, the spin-gravity interaction.
Spin injection into semiconductors
NASA Astrophysics Data System (ADS)
Oestreich, M.; Hübner, J.; Hägele, D.; Klar, P. J.; Heimbrodt, W.; Rühle, W. W.; Ashenford, D. E.; Lunn, B.
1999-03-01
The injection of spin-polarized electrons is presently one of the major challenges in semiconductor spin electronics. We propose and demonstrate a most efficient spin injection using diluted magnetic semiconductors as spin aligners. Time-resolved photoluminescence with a Cd0.98Mn0.02Te/CdTe structure proves the feasibility of the spin-alignment mechanism.
Electrical control of single spin dynamics
NASA Astrophysics Data System (ADS)
Petta, Jason
2012-02-01
Over ten years ago, Daniel Loss and David DiVincenzo proposed using the spin of a single electron as a quantum bit. At the time of the proposal, it was not possible to trap a single electron in a device and measure its spin, let alone demonstrate control of quantum coherence. In this talk I will describe recent progress in the field, focusing on two new methods for single spin control that have been developed by my group at Princeton. The first method is based on quantum interference and implements spin-interferometry on a chip. The second method utilizes the strong spin-orbit coupling of InAs. By shifting the orbital position of the electronic wavefunction at gigahertz frequencies, we can control the orientation of a single electron spin and measure the full g-tensor, which exhibits a large anisotropy due to spin-orbit interactions. Both methods for single spin control are orders of magnitude faster than conventional electron spin resonance and allow investigations of single spin coherence in the presence of fluctuating nuclear and spin-orbit fields. I will also describe recent efforts to transfer these methods to silicon quantum dots, where the effects of fluctuating nuclear fields are much smaller.
Spin-crossover molecule based thermoelectric junction
Ghosh, Dibyajyoti; Parida, Prakash; Pati, Swapan K.
2015-05-11
Using ab-initio numerical methods, we explore the spin-dependent transport and thermoelectric properties of a spin-crossover molecule (i.e., iron complex of 2-(1H-pyrazol-1-yl)-6-(1H-tetrazole-5-yl)pyridine) based nano-junction. We demonstrate a large magnetoresistance, efficient conductance-switching, and spin-filter activity in this molecule-based two-terminal device. The spin-crossover process also modulates the thermoelectric entities. It can efficiently switch the magnitude as well as spin-polarization of the thermocurrent. We find that thermocurrent is changed by ∼4 orders of magnitude upon spin-crossover. Moreover, it also substantially affects the thermopower and consequently, the device shows extremely efficient spin-crossover magnetothermopower generation. Furthermore, by tuning the chemical potential of electrodes into a certain range, a pure spin-thermopower can be achieved for the high-spin state. Finally, the reasonably large values of figure-of-merit in the presence and absence of phonon demonstrate a large heat-to-voltage conversion efficiency of the device. We believe that our study will pave an alternative way of tuning the transport and thermoelectric properties through the spin-crossover process and can have potential applications in generation of spin-dependent current, information storage, and processing.
Transport and spin conversion of multicarriers in semimetal bismuth
NASA Astrophysics Data System (ADS)
Emoto, Hiroyuki; Ando, Yuichiro; Eguchi, Gaku; Ohshima, Ryo; Shikoh, Eiji; Fuseya, Yuki; Shinjo, Teruya; Shiraishi, Masashi
2016-05-01
In this paper, we report on the investigation of (i) the transport properties of multicarriers in semimetal Bi and (ii) the spin conversion physics in this semimetal system on a ferrimagnetic insulator, yttrium-iron-garnet. Hall measurements reveal that electrons and holes coexist in the Bi, with electrons being the dominant carrier. The results of a spin conversion experiment corroborate the results of the Hall measurement; in addition, the inverse spin Hall effect governs the spin conversion in the semimetal/insulator system. This study provides further insights into spin conversion physics in semimetal systems.
Momentum-dependent band spin splitting in semiconducting MnO2: a density functional calculation.
Noda, Yusuke; Ohno, Kaoru; Nakamura, Shinichiro
2016-05-11
Recently, manganese-oxide compounds have attracted considerable attention, in particular, as candidate materials for photochemical water-splitting reactions. Here, we investigate electronic states of pristine manganese dioxides (MnO2) in different crystal phases using spin-polarized density functional theory (DFT) with Hubbard U correction. Geometrical structures and band dispersions of α-, β-, δ-, and λ-MnO2 crystals with collinear magnetic [ferromagnetic (FM) and antiferromagnetic (AFM)] orders are discussed in detail. We reveal that penalty energies that arise by violating the Goodenough-Kanamori rule are important and the origin of the magnetic interactions of the MnO2 crystals is governed by the superexchange interactions of Mn-O-Mn groups. In addition, it is found that momentum-dependent band spin splitting occurs in the AFM α-, β-, and δ-MnO2 crystals while no spin splitting occurs in the AFM λ-MnO2 crystal. Our results show that spin-split band dispersions stem from the different orientations of Mn-centred oxygen octahedra. Such interesting electronic states of the MnO2 crystals are unraveled by our discussion on the relationship between the effective (spin-dependent) single-electron potentials and the space-group symmetry operations that map up-spin Mn atoms onto down-spin Mn atoms. This work provides a basis to understand the relationship between the spin-dependent electronic states and the crystallography of manganese oxides. Another relationship to the recent experimental observations of the photochemical oxygen evolution of MnO2 crystals is also discussed. PMID:27119122
NASA Astrophysics Data System (ADS)
Alday, Luis F.; Bissi, Agnese; Lukowski, Tomasz
2015-11-01
Using conformal field theory (CFT) arguments we derive an infinite number of constraints on the large spin expansion of the anomalous dimensions and structure constants of higher spin operators. These arguments rely only on analyticity, unitarity, crossing-symmetry and the structure of the conformal partial wave expansion. We obtain results for both, perturbative CFT to all order in the perturbation parameter, as well as non-perturbatively. For the case of conformal gauge theories this provides a proof of the reciprocity principle to all orders in perturbation theory and provides a new "reciprocity" principle for structure constants. We argue that these results extend also to non-conformal theories.
NASA Technical Reports Server (NTRS)
Lee, Seungwon; vonAllmen, Paul; Oyafuso, Fabiano; Klimeck, Gerhard; Whale, K. Birgitta
2004-01-01
Electron spin dephasing and decoherence by its interaction with nuclear spins in self-assembled quantum dots are investigated in the framework of the empirical tight-binding model. Electron spin dephasing in an ensemble of dots is induced by the inhomogeneous precession frequencies of the electron among dots, while electron spin decoherence in a single dot arises from the inhomogeneous precession frequencies of nuclear spins in the dot. For In(x)Ga(1-x) As self-assembled dots containing 30000 nuclei, the dephasing and decoherence times are predicted to be on the order of 100 ps and 1 (micro)s.
ADM canonical formalism for gravitating spinning objects
Steinhoff, Jan; Schaefer, Gerhard; Hergt, Steven
2008-05-15
In general relativity, systems of spinning classical particles are implemented into the canonical formalism of Arnowitt, Deser, and Misner [R. Arnowitt, S. Deser, and C. W. Misner, in Gravitation: An Introduction to Current Research, edited by L. Witten (Wiley, New York, 1962), p. 227; arXiv:gr-qc/0405109]. The implementation is made with the aid of a symmetric stress-energy tensor and not a 4-dimensional covariant action functional. The formalism is valid to terms linear in the single spin variables and up to and including the next-to-leading order approximation in the gravitational spin-interaction part. The field-source terms for the spinning particles occurring in the Hamiltonian are obtained from their expressions in Minkowski space with canonical variables through 3-dimensional covariant generalizations as well as from a suitable shift of projections of the curved spacetime stress-energy tensor originally given within covariant spin supplementary conditions. The applied coordinate conditions are the generalized isotropic ones introduced by Arnowitt, Deser, and Misner. As applications, the Hamiltonian of two spinning compact bodies with next-to-leading order gravitational spin-orbit coupling, recently obtained by Damour, Jaranowski, and Schaefer [Phys. Rev. D 77, 064032 (2008)], is rederived and the derivation of the next-to-leading order gravitational spin(1)-spin(2) Hamiltonian, shown for the first time in [J. Steinhoff, S. Hergt, and G. Schaefer, Phys. Rev. D 77, 081501(R) (2008)], is presented.
Symmetry of Magnetically Ordered Quasicrystals
NASA Astrophysics Data System (ADS)
Lifshitz, Ron
1998-03-01
The notion of magnetic symmetry is reexamined in light of the recent observation of long-range magnetic order in icosahedral quasicrystals [Charrier et al., Phys. Rev. Lett. 78, 4637 (1997)]. The relation between the symmetry of a magnetically ordered (periodic or quasiperiodic) crystal, given in terms of a ``spin space group,'' and its neutron diffraction diagram is established. In doing so, an outline of a symmetry classification scheme for magnetically ordered quasiperiodic crystals, is provided. Predictions are given for the expected diffraction patterns of magnetically ordered icosahedral crystals, provided their symmetry is well described by icosahedral spin space groups.
Spin-bowling in cricket re-visited: model trajectories for various spin-vector angles
NASA Astrophysics Data System (ADS)
Robinson, Garry; Robinson, Ian
2016-08-01
In this paper we investigate, via the calculation of model trajectories appropriate to slow bowling in cricket, the effects on the flight path of the ball before pitching due to changes in the angle of the spin-vector. This was accomplished by allowing the spin-vector to vary in three ways. Firstly, from off-spin, where the spin-vector points horizontally and directly down the pitch, to top-spin where it points horizontally towards the off-side of the pitch. Secondly, from off-spin to side-spin where, for side-spin, the spin-vector points vertically upwards. Thirdly, where the spin-vector points horizontally and at 45° to the pitch (in the general direction of ‘point’, as viewed by the bowler), and is varied towards the vertical, while maintaining the 45° angle in the horizontal plane. It is found that, as is well known, top-spin causes the ball to dip in flight, side-spin causes the ball to move side-ways in flight and, perhaps most importantly, off-spin can cause the ball to drift to the off-side of the pitch late in its flight as it begins to fall. At a more subtle level it is found that, if the total spin is kept constant and a small amount of top-spin is added to the ball at the expense of some off-spin, there is little change in the side-ways drift. However, a considerable reduction in the length at which the ball pitches occurs, ∼25 cm, an amount that batsmen can ignore at their peril. On the other hand, a small amount of side-spin introduced to a top-spin delivery does not alter the point of pitching significantly, but produces a considerable amount of side-ways drift, ∼10 cm or more. For pure side-spin the side-ways drift is up to ∼30 cm. When a side-spin component is added to the spin of a ball bowled with a mixture of off-spin and top-spin in equal proportions, significant movement occurs in both the side-ways direction and in the point of pitching, of the order of a few tens of centimetres.
Macroscopic quantum spin tunneling with two interacting spins
NASA Astrophysics Data System (ADS)
Owerre, Solomon A.; Paranjape, M. B.
2013-12-01
We study the simple Hamiltonian, H=-K(S1z2+S2z2)+λS⃗1·S⃗2, of two large, coupled spins which are taken equal, each of total spin s with λ the exchange coupling constant. The exact ground state of this simple Hamiltonian is not known for an antiferromagnetic coupling corresponding to the λ>0. In the absence of the exchange interaction, the ground state is fourfold degenerate, corresponding to the states where the individual spins are in their highest weight or lowest weight states, |↑,↑>,|↓,↓>,|↑,↓>,|↓,↑>, in obvious notation. The first two remain exact eigenstates of the full Hamiltonian. However, we show that the two states |↑,↓>,|↓,↑> organize themselves into the combinations |±>=(1)/(2)(|↑,↓>±|↓↑>), up to perturbative corrections. For the antiferromagnetic case, we show that the ground state is nondegenerate, and we find the interesting result that for integer spins the ground state is |+> and the first excited state is the antisymmetric combination |-> while for half odd integer spin, these roles are exactly reversed. The energy splitting, however, is proportional to λ2s, as expected by perturbation theory to the 2sth order. We obtain these results through the spin coherent state path integral.
Eccentric motion of spinning compact binaries
NASA Astrophysics Data System (ADS)
Tessmer, Manuel; Schäfer, Gerhard
2014-05-01
The equations of motion for spinning compact binaries on eccentric orbits are treated perturbatively in powers of a fractional mass-difference ordering parameter. The solution is valid through first order in the mass-difference parameter. A canonical point transformation removes the leading-order terms of the spin-orbit Hamiltonian which induce a wiggling precession of the orbital angular momentum around the conserved total angular momentum, a precession which disappears in the case of equal masses or one single spin. Action-angle variables are applied that make a canonical perturbation theory easily treatable.
High spin isomer beam line at RIKEN
Kishida, T.; Ideguchi, E.; Wu, H.Y.
1996-12-31
Nuclear high spin states have been the subject of extensive experimental and theoretical studies. For the production of high spin states, fusion reactions are usually used. The orbital angular momentum brought in the reaction is changed into the nuclear spin of the compound nucleus. However, the maximum induced angular momentum is limited in this mechanism by the maximum impact parameter of the fusion reaction and by the competition with fission reactions. It is, therefore, difficult to populate very high spin states, and as a result, large {gamma}-detector arrays have been developed in order to detect subtle signals from such very high spin states. The use of high spin isomers in the fusion reactions can break this limitation because the high spin isomers have their intrinsic angular momentum, which can bring the additional angular momentum without increasing the excitation energy. There are two methods to use the high spin isomers for secondary reactions: the use of the high spin isomers as a target and that as a beam. A high spin isomer target has already been developed and used for several experiments. But this method has an inevitable shortcoming that only {open_quotes}long-lived{close_quotes} isomers can be used for a target: {sup 178}Hf{sup m2} (16{sup +}) with a half-life of 31 years in the present case. By developing a high spin isomer beam, the authors can utilize various short-lived isomers with a short half-life around 1 {mu}s. The high spin isomer beam line of RIKEN Accelerator Facility is a unique apparatus in the world which provides a high spin isomer as a secondary beam. The combination of fusion-evaporation reaction and inverse kinematics are used to produce high spin isomer beams; in particular, the adoption of `inverse kinematics` is essential to use short-lived isomers as a beam.
Spin-Hall effects in metallic antiferromagnets
NASA Astrophysics Data System (ADS)
Zhang, Wei
Materials possessing new parameters for efficient and tunable spin Hall effects are being explored, among which antiferromagnets have become one of the most promising candidates. Two distinct properties of antiferromagnets are the microscopic spin magnetic moment ordering and the intrinsic anisotropy. Thus the natural question arises whether these two unique features of antiferromagnets can become new degrees of freedom for tuning their spin Hall effects. We performed experimental studies using spin pumping and inverse spin Hall detection on prototypical CuAu-I-type metallic antiferromagnets, PtMn, IrMn, PdMn, and FeMn, in which we observed increasing spin Hall effects for the alloys with heavier elements included. In particular, PtMn shows a large spin Hall effect that is comparable to Pt. We also demonstrated that the spin transfer torques from the antiferromagnets are large enough to excite ferromagnetic resonance of an adjacent ferromagnetic layer. We conclude that the sign and magnitude of the spin Hall effects in these antiferromagnets are determined by the atomic spin-orbit coupling of the heavy elements (e.g. Pt and Ir) as well as the large spin magnetic moments of Mn. In addition, by using epitaxial growth, we investigated the influence of the different crystalline and magnetic orientations on the anisotropic spin Hall effects of these antiferromagnets. Most of the experimental results were further corroborated by first-principles calculations, which determine the intrinsic spin Hall effect contribution and suggest pronounced anisotropies. Thus metallic antiferromagnets may become an active component for manipulating spin dependent transport properties in spintronic concepts. Work at Argonne was supported by the U.S. DOE, OS, Materials Sciences and Engineering Division. Work at Center for Nanoscale Materials was supported by DOE, OS-BES (DE-AC02-06CH11357). Work at Julich was supported by SPP 1538 Programme of the DFG.
Tidal deformations of a spinning compact object
NASA Astrophysics Data System (ADS)
Pani, Paolo; Gualtieri, Leonardo; Maselli, Andrea; Ferrari, Valeria
2015-07-01
The deformability of a compact object induced by a perturbing tidal field is encoded in the tidal Love numbers, which depend sensibly on the object's internal structure. These numbers are known only for static, spherically-symmetric objects. As a first step to compute the tidal Love numbers of a spinning compact star, here we extend powerful perturbative techniques to compute the exterior geometry of a spinning object distorted by an axisymmetric tidal field to second order in the angular momentum. The spin of the object introduces couplings between electric and magnetic deformations and new classes of induced Love numbers emerge. For example, a spinning object immersed in a quadrupolar, electric tidal field can acquire some induced mass, spin, quadrupole, octupole and hexadecapole moments to second order in the spin. The deformations are encoded in a set of inhomogeneous differential equations which, remarkably, can be solved analytically in vacuum. We discuss certain subtleties in defining the tidal Love numbers in general relativity, which are due to the difficulty in separating the tidal field from the linear response of the object in the solution, even in the static case. By extending the standard procedure to identify the linear response in the static case, we prove analytically that the Love numbers of a Kerr black hole remain zero to second order in the spin. As a by-product, we provide the explicit form for a slowly-rotating, tidally-deformed Kerr black hole to quadratic order in the spin, and discuss its geodesic and geometrical properties.
Zhang, Wei; Jungfleisch, Matthias B.; Freimuth, Frank; Jiang, Wanjun; Sklenar, Joseph; Pearson, John E.; Ketterson, John B.; Mokrousov, Yuri; Hoffmann, Axel
2015-10-06
We investigate spin-orbit torques of metallic CuAu-I-type antiferromagnets using spin-torque ferromagnetic resonance tuned by a dc-bias current. The observed spin torques predominantly arise from diffusive transport of spin current generated by the spin Hall effect. We find a growth-orientation dependence of the spin torques by studying epitaxial samples, which may be correlated to the anisotropy of the spin Hall effect. The observed anisotropy is consistent with first-principles calculations on the intrinsic spin Hall effect. Our work suggests large tunable spin-orbit effects in magnetically-ordered materials.
Nuclear spin circular dichroism
Vaara, Juha; Rizzo, Antonio; Kauczor, Joanna; Norman, Patrick; Coriani, Sonia
2014-04-07
Recent years have witnessed a growing interest in magneto-optic spectroscopy techniques that use nuclear magnetization as the source of the magnetic field. Here we present a formulation of magnetic circular dichroism (CD) due to magnetically polarized nuclei, nuclear spin-induced CD (NSCD), in molecules. The NSCD ellipticity and nuclear spin-induced optical rotation (NSOR) angle correspond to the real and imaginary parts, respectively, of (complex) quadratic response functions involving the dynamic second-order interaction of the electron system with the linearly polarized light beam, as well as the static magnetic hyperfine interaction. Using the complex polarization propagator framework, NSCD and NSOR signals are obtained at frequencies in the vicinity of optical excitations. Hartree-Fock and density-functional theory calculations on relatively small model systems, ethene, benzene, and 1,4-benzoquinone, demonstrate the feasibility of the method for obtaining relatively strong nuclear spin-induced ellipticity and optical rotation signals. Comparison of the proton and carbon-13 signals of ethanol reveals that these resonant phenomena facilitate chemical resolution between non-equivalent nuclei in magneto-optic spectra.
Silicon-on-insulator for spintronic applications: spin lifetime and electric spin manipulation
NASA Astrophysics Data System (ADS)
Sverdlov, Viktor; Osintsev, Dmitri; Selberherr, Siegfried
2016-05-01
With complementary metal-oxide semiconductor feature size rapidly approaching ultimate scaling limits, the electron spin attracts much attention as an alternative to the electron charge degree of freedom for low-power reprogrammable logic and nonvolatile memory applications. Silicon, the main element of microelectronics, appears to be the perfect material for spin-driven applications. Despite an impressive progress in understanding spin properties in metal-oxide-semiconductor field-effect transistors (MOSFETs), spin manipulation in a silicon channel by means of the electric field-dependent Rashba-like spin-orbit interaction requires channels much longer than 20 nm channel length of modern MOSFETs. Although a successful realization of the spin field-effect transistor seems to be unlikely without a new concept for an efficient way of spin manipulation in silicon by purely electrical means, it is demonstrated that shear strain dramatically reduces the spin relaxation, thus boosting the spin lifetime by an order of magnitude. Spin lifetime enhancement is achieved by lifting the degeneracy between the otherwise equivalent unprimedsubbands by [110] uniaxial stress. The spin lifetime in stressed ultra-thin body silicon-on-insulator structures can reach values close to those in bulk silicon. Therefore, stressed silicon-on-insulator structures have a potential for spin interconnects.
Spin-current noise from fluctuation relations
Lim, Jong Soo; Sánchez, David; López, Rosa
2013-12-04
We present fluctuation relations that connect spin-polarized current and noise in mesoscopic conductors. In linear response, these relations are equivalent to the fluctuation-dissipation theorem that relates equilibrium current-current correlations to the linear conductance. More interestingly, in the weakly nonlinear regime of transport, these relations establish a connection between the leading-order rectification spin conductance, the spin noise susceptibility and the third cumulant of spin current fluctuations at equilibrium. Our results are valid even for systems in the presence of magnetic fields and coupled to ferromagnetic electrodes.
Spin coupling in zigzag Wigner crystals.
Klironomos, A. D.; Meyer, J. S.; Hikihara, T.; Matveev, K. A.; Materials Science Division; Ohio State Univ.; Hokkaido Univ.
2007-08-01
We consider interacting electrons in a quantum wire in the case of a shallow confining potential and low electron density. In a certain range of densities, the electrons form a two-row (zigzag) Wigner crystal whose spin properties are determined by nearest and next-nearest neighbor exchange as well as by three- and four-particle ring exchange processes. The phase diagram of the resulting zigzag spin chain has regions of complete spin polarization and partial spin polarization in addition to a number of unpolarized phases, including antiferromagnetism and dimer order as well as a novel phase generated by the four-particle ring exchange.
Dynamics of Spin-(1)/(2) Quantum Plasmas
NASA Astrophysics Data System (ADS)
Marklund, Mattias; Brodin, Gert
2007-01-01
The fully nonlinear governing equations for spin-(1)/(2) quantum plasmas are presented. Starting from the Pauli equation, the relevant plasma equations are derived, and it is shown that nontrivial quantum spin couplings arise, enabling studies of the combined collective and spin dynamics. The linear response of the quantum plasma in an electron-ion system is obtained and analyzed. Applications of the theory to solid state and astrophysical systems as well as dusty plasmas are pointed out.
Dynamics of spin-1/2 quantum plasmas.
Marklund, Mattias; Brodin, Gert
2007-01-12
The fully nonlinear governing equations for spin-1/2 quantum plasmas are presented. Starting from the Pauli equation, the relevant plasma equations are derived, and it is shown that nontrivial quantum spin couplings arise, enabling studies of the combined collective and spin dynamics. The linear response of the quantum plasma in an electron-ion system is obtained and analyzed. Applications of the theory to solid state and astrophysical systems as well as dusty plasmas are pointed out. PMID:17358613
Spin decoherence processes in the S = 1/2 scalene triangular cluster (Cu3(OH))
NASA Astrophysics Data System (ADS)
Ponomaryov, A. N.; Kim, N.; Jang, Z. H.; van Tol, J.; Koo, H.-J.; Law, J. M.; Suh, B. J.; Yoon, S.; Choi, K. Y.
2015-03-01
We report the synthesis and magnetic properties of the molecular cluster Cu3({{μ }3}-OH)(μ-OH)(μ-O2Ar4F-Ph)2(py)3(OTf)2, abbreviated as (Cu3(OH)). Using magnetization, electron paramagnetic resonance and spin dimer analysis, we derive a microscopic magnetic model of (Cu3(OH)) and measure the electron T1 and T2 relaxation times. The Cu2+ ions are arranged to form a distorted triangular structure with the three different exchange coupling constants {{J}1}=-43.5 K, {{J}2}=-53.0 K, and {{J}3}=-37.7 K. At T = 1.5 K T1 is of the order of 10-4 s and T2 is evaluated to be 0.26 μ s. We find that the temperature dependence of 1/{{T}1} and 1/{{T}2} is governed by Orbach process and spin bath fluctuations, respectively. We discuss the role of spin-phonon mechanism in determining a spin decoherence time in a class of spin triangular clusters.
Measurement of spin coherence using Raman scattering
NASA Astrophysics Data System (ADS)
Sun, Z.; Delteil, A.; Faelt, S.; Imamoǧlu, A.
2016-06-01
Ramsey interferometry provides a natural way to determine the coherence time of most qubit systems. Recent experiments on quantum dots, however, demonstrated that dynamical nuclear spin polarization can strongly influence the measurement process, making it difficult to extract the T2* coherence time using standard optical Ramsey pulses. Here, we demonstrate an alternative method for spin coherence measurement that is based on first-order coherence of photons generated in spin-flip Raman scattering. We show that if a quantum emitter is driven by a weak monochromatic laser, Raman coherence is determined exclusively by spin coherence, allowing for a direct determination of spin T2* time. When combined with coherence measurements on Rayleigh scattered photons, our technique enables us to identify coherent and incoherent contributions to resonance fluorescence, and to minimize the latter. We verify the validity of our technique by comparing our results to those determined from Ramsey interferometry for electron and heavy-hole spins.